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Sample records for 2-dimensional premixed flames

  1. Premixed turbulent flame calculation

    NASA Technical Reports Server (NTRS)

    El-Tahry, S.; Rutland, C. J.; Ferziger, J. H.; Rogers, M. M.

    1987-01-01

    The importance of turbulent premixed flames in a variety of applications has led to a substantial amount of effort towards improving the understanding of these flames. Although these efforts have increased the understanding, many questions still remain. The use of direct numerical simulation (DNS) in solving these questions is examined.

  2. Simultaneous measurement of 2-dimensional H2O concentration and temperature distribution in premixed methane/air flame using TDLAS-based tomography technology

    NASA Astrophysics Data System (ADS)

    Wang, Fei; Wu, Qi; Huang, Qunxing; Zhang, Haidan; Yan, Jianhua; Cen, Kefa

    2015-07-01

    An innovative tomographic method using tunable diode laser absorption spectroscopy (TDLAS) and algebraic reconstruction technique (ART) is presented in this paper for detecting two-dimensional distribution of H2O concentration and temperature in a premixed flame. The collimated laser beam emitted from a low cost diode laser module was delicately split into 24 sub-beams passing through the flame from different angles and the acquired laser absorption signals were used to retrieve flame temperature and H2O concentration simultaneously. The efficiency of the proposed reconstruction system and the effect of measurement noise were numerically evaluated. The temperature and H2O concentration in flat methane/air premixed flames under three different equivalence ratios were experimentally measured and reconstruction results were compared with model calculations. Numerical assessments indicate that the TDLAS tomographic system is capable for temperature and H2O concentration profiles detecting even the noise strength reaches 3% of absorption signal. Experimental results under different combustion conditions are well demonstrated along the vertical direction and the distribution profiles are in good agreement with model calculation. The proposed method exhibits great potential for 2-D or 3-D combustion diagnostics including non-uniform flames.

  3. Statistics of premixed flame cells

    NASA Technical Reports Server (NTRS)

    Noever, David A.

    1991-01-01

    The statistics of random cellular patterns in premixed flames are analyzed. Agreement is found with a variety of topological relations previously found for other networks, namely, Lewis's law and Aboav's law. Despite the diverse underlying physics, flame cells are shown to share a broad class of geometric properties with other random networks-metal grains, soap foams, bioconvection, and Langmuir monolayers.

  4. Statistics of premixed flame cells

    SciTech Connect

    Noever, D.A. )

    1991-07-15

    The statistics of random cellular patterns in premixed flames are analyzed. Agreement is found with a variety of topological relations previously found for other networks, namely, Lewis's law and Aboav's law. Despite the diverse underlying physics, flame cells are shown to share a broad class of geometric properties with other random networks---metal grains, soap foams, bioconvection, and Langmuir monolayers.

  5. Flame front configuration of turbulent premixed flames

    SciTech Connect

    Furukawa, Junichi; Maruta, Kaoru; Hirano, Toshisuke

    1998-02-01

    The present study is performed to explore dependence of the wrinkle scale of propane-air turbulent premixed flames on the characteristics of turbulence in the nonreacting flow, burner size, and mixture ratio. The wrinkle scales are examined and expressed in the frequency distribution of the radii of flame front curvatures. The average wrinkle scale depends not only on the characteristics of turbulence in the nonreacting flow but also on burner diameter and mixture ratio. The average wrinkle scale of a lean propane-air flame is larger than those of the near stoichiometric and rich flames. The smallest wrinkle scale of turbulent premixed flame is in the range of 0.75--1.0 mm, which is much larger than the Kolmogorov scale of turbulence in the nonreacting flow.

  6. Flame front geometry in premixed turbulent flames

    SciTech Connect

    Shepherd, I.G. ); Ashurst, W.T. )

    1991-12-01

    Experimental and numerical determinations of flame front curvature and orientation in premixed turbulent flames are presented. The experimental data is obtained from planar, cross sectional images of stagnation point flames at high Damkoehler number. A direct numerical simulation of a constant energy flow is combined with a zero-thickness, constant density flame model to provide the numerical results. The computational domain is a 32{sup 3} cube with periodic boundary conditions. The two-dimensional curvature distributions of the experiments and numerical simulations compare well at similar q{prime}/S{sub L} values with means close to zero and marked negative skewness. At higher turbulence levels the simulations show that the distributions become symmetric about zero. These features are also found in the three dimensional distributions of curvature. The simulations support assumptions which make it possible to determine the mean direction cosines from the experimental data. This leads to a reduction of 12% in the estimated flame surface area density in the middle of the flame brush. 18 refs.

  7. Studies of Premixed Laminar and Turbulent Flames at Microgravity

    NASA Technical Reports Server (NTRS)

    Abid, M.; Aung, K.; Ronney, P. D.; Sharif, J. A.; Wu, M.-S.

    1999-01-01

    Several topics relating to combustion limits in premixed flames at reduced gravity have been studied. These topics include: (1) flame balls; (2) numerical simulation of flame ball and planar flame structure and stability; (3) experimental simulation of buoyancy effects in premixed flames using aqueous autocatalytic reactions; and (4) premixed flame propagation in Hele-Shaw cells.

  8. Soot Formation in Laminar Premixed Flames

    NASA Technical Reports Server (NTRS)

    Xu, F.; Krishnan, S. S.; Faeth, G. M.

    1999-01-01

    Soot processes within hydrocarbon-fueled flames affect emissions of pollutant soot, thermal loads on combustors, hazards of unwanted fires and capabilities for computational combustion. In view of these observations, the present study is considering processes of soot formation in both burner-stabilized and freely-propagating laminar premixed flames. These flames are being studied in order to simplify the interpretation of measurements and to enhance computational tractability compared to the diffusion flame environments of greatest interest for soot processes. In addition, earlier studies of soot formation in laminar premixed flames used approximations of soot optical and structure properties that have not been effective during recent evaluations, as well as questionable estimates of flow residence times). The objective of present work was to exploit methods of avoiding these difficulties developed for laminar diffusion flames to study soot growth in laminar premixed flames. The following description of these studies is brief.

  9. Premixed turbulent flame propagation in microgravity

    NASA Technical Reports Server (NTRS)

    Menon, S.; Jagoda, J.; Sujith, R.

    1995-01-01

    To reduce pollutant formation there is, at present, an increased interest in employing premixed fuel/air mixture in combustion devices. It is well known that greater control over local temperature can be achieved with premixed flames and with lean premixed mixtures, significant reduction of pollutants such as NO(x) can be achieved. However, an issue that is still unresolved is the predictability of the flame propagation speed in turbulent premixed mixtures, especially in lean mixtures. Although substantial progress has been made in recent years, there is still no direct verification that flame speeds in turbulent premixed flows are highly predictable in complex flow fields found in realistic combustors. One of the problems associated with experimental verification is the difficulty in obtaining access to all scales of motion in typical high Reynolds number flows, since, such flows contain scales of motion that range from the size of the device to the smallest Kolmogorov scale. The overall objective of this study is to characterize the behavior of turbulent premixed flames at reasonable high Reynolds number, Re(sub L). Of particular interest here is the thin flame limit where the laminar flame thickness is much smaller than the Kolmogorov scale. Thin flames occur in many practical combustion devices and will be numerically studied using a recently developed new formulation that is briefly described.

  10. Lifted Partially Premixed Flames in Microgravity

    NASA Technical Reports Server (NTRS)

    Lock, Andrew J.; Ganguly, Ranjan; Puri, Ishwar K.; Aggarwal, Suesh K.; Hegde, Uday

    2004-01-01

    Lifted Double and Triple flames are established in the UIC-NASA Partially Premixed microgravity rig. The flames examined in this paper are established above a coannular burner because its axisymmetric geometry allows for future implementation of other non-intrusive optical diagnostic techniques easily. Both burner-attached stable flames and lifted flames are established at normal and microgravity conditions in the drop tower facility.

  11. Displacement speeds in turbulent premixed flame simulations

    SciTech Connect

    Day, Marcus S.; Shepherd, Ian G.; Bell, J.; Grcar, Joseph F.; Lijewski, Michael J.

    2007-07-01

    The theory of turbulent premixed flames is based on acharacterization of the flame as a discontinuous surface propagatingthrough the fluid. The displacement speed, defined as the local speed ofthe flame front normal to itself, relative to the unburned fluid,provides one characterization of the burning velocity. In this paper, weintroduce a geometric approach to computing displacement speed anddiscuss the efficacy of the displacement speed for characterizing aturbulent flame.

  12. Flame propagation in partially premixed conditions

    NASA Astrophysics Data System (ADS)

    Ruetsch, G.; Poinsot, T.; Veynante, D.; Trouvé, A.

    1996-11-01

    Turbulent flame propagation is studied under inhomogenously premixed conditions via data from direct numerical simulations. Departures from the premixed case are studied using four different configurations, ranging from one dimensional unsteady flames to turbulent three-dimensional simulations. Simulations are performed in these cases with various values of the mean equivalence ratio, fluctuations about the mean equivlalence ratio, correlation length scales, and probability denisty functions of the mixture composition. Propagation characteristics are described in terms of the flamelet approach, where the the main contribution of partial premixing on flame propagation is due to flame wrinkling relative to modification of the mean flamelet structure. This behavior is consistent over a broad range of conditions, with the exception being extreme departures from stoichiometric conditions where flamability limits are exceeded and flame quenching is observed.

  13. Turbulent Premixed Flames in Microgravity

    NASA Technical Reports Server (NTRS)

    Menon, Suresh

    1996-01-01

    The experimental cold-flow facility is now full operational and is currently being used to obtain baseline turbulence data in a Couette flow. The baseline turbulence data is necessary to confirm the capability of the chosen device to generate and maintain the required turbulence intensity. Subsequent reacting flow studies will assume that a similar turbulent flow field exists ahead of the premixed flame. Some modifications and refinements had to be made to enable accurate measurements. It consists of two rollers, one (driven by a motor) which drives a continuous belt and four smaller rollers used to set the belt spacing and tension to minimize belt flutter. The entire assemble is enclosed in a structure that has the dimensions to enable future drop tower experiments of the hot facility. All critical dimensions are the same as the original plans except for the pulley ratio which has been changed to enable a wider operating regime in terms of the Reynolds number. With the current setup, Reynolds numbers as low as 100 and as high as 14,000 can be achieved. This is because the in-between belt spacing can be varied from 1 cm to 7.6 cm, and the belt speed can be accurately varied from .15 m/sec to 3.1 m/sec.

  14. Dynamics and structure of turbulent premixed flames

    NASA Technical Reports Server (NTRS)

    Bilger, R. W.; Swaminathan, N.; Ruetsch, G. R.; Smith, N. S. A.

    1995-01-01

    In earlier work (Mantel & Bilger, 1994) the structure of the turbulent premixed flame was investigated using statistics based on conditional averaging with the reaction progress variable as the conditioning variable. The DNS data base of Trouve and Poinsot (1994) was used in this investigation. Attention was focused on the conditional dissipation and conditional axial velocity in the flame with a view to modeling these quantities for use in the conditional moment closure (CMC) approach to analysis of kinetics in premixed flames (Bilger, 1993). Two remarkable findings were made: there was almost no acceleration of the axial velocity in the flame front itself; and the conditional scalar dissipation remained as high, or higher, than that found in laminar premixed flames. The first finding was surprising since in laminar flames all the fluid acceleration occurs through the flame front, and this could be expected also for turbulent premixed flames at the flamelet limit. The finding gave hope of inventing a new approach to the dynamics of turbulent premixed flames through use of rapid distortion theory or an unsteady Bernoulli equation. This could lead to a new second order closure for turbulent premixed flames. The second finding was contrary to our measurements with laser diagnostics in lean hydrocarbon flames where it is found that conditional scalar dissipation drops dramatically below that for laminar flamelets when the turbulence intensity becomes high. Such behavior was not explainable with a one-step kinetic model, even at non-unity Lewis number. It could be due to depletion of H2 from the reaction zone by preferential diffusion. The capacity of the flame to generate radicals is critically dependent on the levels of H2 present (Bilger, et al., 1991). It seemed that a DNS computation with a multistep reduced mechanism would be worthwhile if a way could be found to make this feasible. Truly innovative approaches to complex problems often come only when there is the

  15. Studies of Premixed Laminar and Turbulent Flames at Microgravity

    NASA Technical Reports Server (NTRS)

    Kwon, O. C.; Abid, M.; Porres, J.; Liu, J. B.; Ronney, P. D.; Struk, P. M.; Weiland, K. J.

    2003-01-01

    Several topics relating to premixed flame behavior at reduced gravity have been studied. These topics include: (1) flame balls; (2) flame structure and stability at low Lewis number; (3) experimental simulation of buoyancy effects in premixed flames using aqueous autocatalytic reactions; and (4) premixed flame propagation in Hele-Shaw cells. Because of space limitations, only topic (1) is discussed here, emphasizing results from experiments on the recent STS-107 Space Shuttle mission, along with numerical modeling efforts.

  16. Premixed Turbulent Flame Propagation in Microgravity

    NASA Technical Reports Server (NTRS)

    Menon, Suresh

    1999-01-01

    A combined numerical-experimental study has been carried out to investigate the structure and propagation characteristics of turbulent premixed flames with and without the influence of buoyancy. Experimentally, the premixed flame characteristics are studied in the wrinkled regime using a Couette flow facility and an isotropic flow facility in order to resolve the scale of flame wrinkling. Both facilities were chosen for their ability to achieve sustained turbulence at low Reynolds number. This implies that conventional diagnostics can be employed to resolve the smallest scales of wrinkling. The Couette facility was also built keeping in mind the constraints imposed by the drop tower requirements. Results showed that the flow in this Couette flow facility achieves full-developed turbulence at low Re and all turbulence statistics are in good agreement with past measurements on large-scale facilities. Premixed flame propagation studies were then carried out both using the isotropic box and the Couette facility. Flame imaging showed that fine scales of wrinkling occurs during flame propagation. Both cases in Ig showed significant buoyancy effect. To demonstrate that micro-g can remove this buoyancy effect, a small drop tower was built and drop experiments were conducted using the isotropic box. Results using the Couette facility confirmed the ability to carry out these unique reacting flow experiments at least in 1g. Drop experiments at NASA GRC were planned but were not completed due to termination of this project.

  17. Premixed flame propagation in vertical tubes

    NASA Astrophysics Data System (ADS)

    Kazakov, Kirill A.

    2016-04-01

    Analytical treatment of the premixed flame propagation in vertical tubes with smooth walls is given. Using the on-shell flame description, equations for a quasi-steady flame with a small but finite front thickness are obtained and solved numerically. It is found that near the limits of inflammability, solutions describing upward flame propagation come in pairs having close propagation speeds and that the effect of gravity is to reverse the burnt gas velocity profile generated by the flame. On the basis of these results, a theory of partial flame propagation driven by a strong gravitational field is developed. A complete explanation is given of the intricate observed behavior of limit flames, including dependence of the inflammability range on the size of the combustion domain, the large distances of partial flame propagation, and the progression of flame extinction. The role of the finite front-thickness effects is discussed in detail. Also, various mechanisms governing flame acceleration in smooth tubes are identified. Acceleration of methane-air flames in open tubes is shown to be a combined effect of the hydrostatic pressure difference produced by the ambient cold air and the difference of dynamic gas pressure at the tube ends. On the other hand, a strong spontaneous acceleration of the fast methane-oxygen flames at the initial stage of their evolution in open-closed tubes is conditioned by metastability of the quasi-steady propagation regimes. An extensive comparison of the obtained results with the experimental data is made.

  18. Active control for turbulent premixed flame simulations

    SciTech Connect

    Bell, John B.; Day, Marcus S.; Grcar, Joseph F.; Lijewski, Michael J.

    2004-03-26

    Many turbulent premixed flames of practical interest are statistically stationary. They occur in combustors that have anchoring mechanisms to prevent blow-off and flashback. The stabilization devices often introduce a level of geometric complexity that is prohibitive for detailed computational studies of turbulent flame dynamics. As a result, typical detailed simulations are performed in simplified model configurations such as decaying isotropic turbulence or inflowing turbulence. In these configurations, the turbulence seen by the flame either decays or, in the latter case, increases as the flame accelerates toward the turbulent inflow. This limits the duration of the eddy evolutions experienced by the flame at a given level of turbulent intensity, so that statistically valid observations cannot be made. In this paper, we apply a feedback control to computationally stabilize an otherwise unstable turbulent premixed flame in two dimensions. For the simulations, we specify turbulent in flow conditions and dynamically adjust the integrated fueling rate to control the mean location of the flame in the domain. We outline the numerical procedure, and illustrate the behavior of the control algorithm. We use the simulations to study the propagation and the local chemical variability of turbulent flame chemistry.

  19. Gravity Effects Observed In Partially Premixed Flames

    NASA Technical Reports Server (NTRS)

    Puri, Ishwar K.; Aggarwal, Suresh K.; Lock, Andrew J.; Gauguly, Ranjan; Hegde, Uday

    2003-01-01

    Partially premixed flames (PPFs) contain a rich premixed fuel air mixture in a pocket or stream, and, for complete combustion to occur, they require the transport of oxidizer from an appropriately oxidizer-rich (or fuel-lean) mixture that is present in another pocket or stream. Partial oxidation reactions occur in fuel-rich portions of the mixture and any remaining unburned fuel and/or intermediate species are consumed in the oxidizer-rich portions. Partial premixing, therefore, represents that condition when the equivalence ratio (phi) in one portion of the flowfield is greater than unity, and in another section its value is less than unity. In general, for combustion to occur efficiently, the global equivalence ratio is in the range fuel-lean to stoichiometric. These flames can be established by design by placing a fuel-rich mixture in contact with a fuel-lean mixture, but they also occur otherwise in many practical systems, which include nonpremixed lifted flames, turbulent nonpremixed combustion, spray flames, and unwanted fires. Other practical applications of PPFs are reported elsewhere. Although extensive experimental studies have been conducted on premixed and nonpremixed flames under microgravity, there is a absence of previous experimental work on burner stabilized PPFs in this regard. Previous numerical studies by our group employing a detailed numerical model showed gravity effects to be significant on the PPF structure. We report on the results of microgravity experiments conducted on two-dimensional (established on a Wolfhard-Parker slot burner) and axisymmetric flames (on a coannular burner) that were investigated in a self-contained multipurpose rig. Thermocouple and radiometer data were also used to characterize the thermal transport in the flame.

  20. Premixed flames in closed cylindrical tubes

    NASA Astrophysics Data System (ADS)

    Metzener, Philippe; Matalon, Moshe

    2001-09-01

    We consider the propagation of a premixed flame, as a two-dimensional sheet separating unburned gas from burned products, in a closed cylindrical tube. A nonlinear evolution equation, that describes the motion of the flame front as a function of its mean position, is derived. The equation contains a destabilizing term that results from the gas motion induced by thermal expansion and has a memory term associated with vorticity generation. Numerical solutions of this equation indicate that, when diffusion is stabilizing, the flame evolves into a non-planar form whose shape, and its associated symmetry properties, are determined by the Markstein parameter, and by the initial data. In particular, we observe the development of convex axisymmetric or non-axisymmetric flames, tulip flames and cellular flames.

  1. Can we characterize turbulence in premixed flames?

    SciTech Connect

    Lipatnikov, A.N.

    2009-06-15

    Modeling of premixed turbulent combustion involves averaging reaction rates in turbulent flows. The focus of most approaches to resolving this problem has been placed on determining the dependence of the mean rate w of product creation on the laminar flame speed S{sub L}, the rms turbulence velocity u', etc. The goal of the present work is to draw attention to another issue: May the input quantity u{sup '} for a model of w= w(u'/S{sub L},..) be considered to be known? The point is that heat release substantially affects turbulence and, hence, turbulence characteristics in premixed flames should be modeled. However, standard moment methods for numerically simulating turbulent flows do not allow us to evaluate the true turbulence characteristics in a flame. For instance, the Reynolds stresses in premixed flames are affected not only by turbulence itself, but also by velocity jump across flamelets. A common way to resolving this problem consists of considering the Reynolds stresses conditioned on unburned (or burned) mixture to be the true turbulence characteristics. In the present paper, this widely accepted but never proved hypothesis is put into question, first, by considering simple model constant-density problems (flame motion in an oscillating one-dimensional laminar flow; flame stabilized in a periodic shear, one-dimensional, laminar flow; turbulent mixing). In all the cases, the magnitude of velocity fluctuations, calculated using the conditioned Reynolds stresses, is affected by the intermittency of reactants and products and, hence, is not the true rms velocity. Second, the above claim is further supported by comparing balance equations for the mean and conditioned Reynolds stresses. The conditioned Reynolds stresses do not characterize the true turbulence in flames, because conditional averaging cuts off flow regions characterized by either high or low velocities. (author)

  2. Studies of Premixed Laminar and Turbulent Flames at Microgravity

    NASA Technical Reports Server (NTRS)

    Ronney, Paul D.

    1993-01-01

    The work of the Principal Investigator (PI) has encompassed four topics related to the experimental and theoretical study of combustion limits in premixed flames at microgravity, as discussed in the following sections. These topics include: (1) radiation effects on premixed gas flames; (2) flame structure and stability at low Lewis number; (3) flame propagation and extinction is cylindrical tubes; and (4) experimental simulation of combustion processes using autocatalytic chemical reactions.

  3. Laminar Premixed and Diffusion Flames (Ground-Based Study)

    NASA Technical Reports Server (NTRS)

    Dai, Z.; El-Leathy, A. M.; Lin, K.-C.; Sunderland, P. B.; Xu, F.; Faeth, G. M.; Urban, D. L. (Technical Monitor); Yuan, Z.-G. (Technical Monitor)

    2000-01-01

    Ground-based studies of soot processes in laminar flames proceeded in two phases, considering laminar premixed flames and laminar diffusion flames, in turn. The test arrangement for laminar premixed flames involved round flat flame burners directed vertically upward at atmospheric pressure. The test arrangement for laminar jet diffusion flames involved a round fuel port directed vertically upward with various hydrocarbon fuels burning at atmospheric pressure in air. In both cases, coflow was used to prevent flame oscillations and measurements were limited to the flame axes. The measurements were sufficient to resolve soot nucleation, growth and oxidation rates, as well as the properties of the environment needed to evaluate mechanisms of these processes. The experimental methods used were also designed to maintain capabilities for experimental methods used in corresponding space-based experiments. This section of the report will be limited to consideration of flame structure for both premixed and diffusion flames.

  4. NOx Formation in a Premixed Syngas Flame

    SciTech Connect

    Yilmaz, S.L.; Givi, P.; Strakey, P.; Casleton, K.

    2006-11-01

    Reduction of NOx is a subject of significant current interest in stationary gas turbines. The objective of this study is to examine the effects of turbulence on non-thermal NOx formation in a syngas flame. This is archived by a detailed parametric study via PDF simulations of a partially stirred reactor and a dumped axisymmetric premixed flame. Several different detailed and reduced kinetics schemes are considered. The simulated results demonstrate the strong dependence of combustion process on turbulence. It is shown that the amount of NOx formation is significantly influenced by the inlet conditions. That is, the turbulence intensity can be tweaked to attain optimal ultra-low NOx emissions at a given temperature.

  5. A Method to Measure Flame Index in Turbulent Partially-Premixed Flames

    NASA Astrophysics Data System (ADS)

    Rosenberg, David Ari

    This dissertation describes the development of a diagnostic technique and data processing routine to measure the flame index in partially-premixed flames, called the Flame Index Measurement Method. Many modern combustion applications involve conditions in which the fuel and oxidizer are only partially mixed prior to entering the flame. These partially-premixed flames contain some regions of premixed and some regions of non-premixed flamelets. New computational approaches use the flame index concept: premixed regions are identified and a premixed model is applied; non-premixed regions are also identified and a non-premixed model is applied. The flame index is defined as the normalized dot product of the gradients of the fuel and oxidizer mass fractions; it is +1 in premixed flamelets and is -1 in non-premixed flamelets. Previously there had been no experimentally measured values of flame index available to assess the modeling approaches. A new method has been developed to measure the flame index using planar laser-induced fluorescence tracers to indicate the sign and direction of the fuel and oxygen gradients. Through the modeling of premixed and non-premixed flamelets, acetone was selected as a fuel tracer and nitrogen dioxide was selected as an oxygen tracer. The fluorescence properties of both acetone and nitrogen dioxide were studied. With acetone seeded into the fuel, and nitrogen dioxide seeded into the air, the Flame Index Measurement Method was evaluated in laminar premixed and non-premixed methane/acetone/air flames, as well as in a well-defined turbulent partially-premixed burner, the Gas Turbine Model Combustor (GTMC). The flame index was measured in the GTMC with methane, propane, and syngas flames. Statistics (mean, variance, and probability mass functions) of the flame index are reported for the highly-turbulent partially-premixed GTMC flames. Two new statistical quantities were developed that describe the probability for the occurrence of premixed

  6. Acoustic radiation from weakly wrinkled premixed flames

    SciTech Connect

    Lieuwen, Tim; Mohan, Sripathi; Rajaram, Rajesh; Preetham,

    2006-01-01

    This paper describes a theoretical analysis of acoustic radiation from weakly wrinkled (i.e., u'/S{sub L}<1) premixed flames. Specifically, it determines the transfer function relating the spectrum of the acoustic pressure oscillations, P'({omega}), to that of the turbulent velocity fluctuations in the approach flow, U'({omega}). In the weakly wrinkled limit, this transfer function is local in frequency space; i.e., velocity fluctuations at a frequency {omega} distort the flame and generate sound at the same frequency. This transfer function primarily depends upon the flame Strouhal number St (based on mean flow velocity and flame length) and the correlation length, {lambda}, of the flow fluctuations. For cases where the ratio of the correlation length and duct radius {lambda}/a>>1, the acoustic pressure and turbulent velocity power spectra are related by P'({omega})-{omega}{sup 2}U'({omega}) and P'({omega})-U'({omega}) for St<<1 and St>>1, respectively. For cases where {lambda}/a<<1, the transfer functions take the form P'({omega})-{omega}{sup 2}({lambda}/a){sup 2}U'({omega}) and P'({omega})-{omega}{sup 2}({lambda}/a){sup 2}({psi}-{delta}ln({lambda}/a))U'({omega}) for St<<1 and St>>1, respectively, where (PS) and {delta} are constants. The latter result demonstrates that this transfer function does not exhibit a simple power law relationship in the high frequency region of the spectra. The simultaneous dependence of this pressure-velocity transfer function upon the Strouhal number and correlation length suggests a mechanism for the experimentally observed maximum in acoustic spectra and provides some insight into the controversy in the literature over how this peak should scale with the flame Strouhal number.

  7. Studies of premixed laminar and turbulent flames at microgravity

    NASA Technical Reports Server (NTRS)

    Ronney, Paul D.

    1993-01-01

    A two and one-half year experimental and theoretical research program on the properties of laminar and turbulent premixed gas flames at microgravity was conducted. Progress during this program is identified and avenues for future studies are discussed.

  8. Soot Formation in Freely-Propagating Laminar Premixed Flames

    NASA Technical Reports Server (NTRS)

    Lin, K.-C.; Hassan, M. I.; Faeth, G. M.

    1997-01-01

    Soot formation within hydrocarbon-fueled flames is an important unresolved problem of combustion science. Thus, the present study is considering soot formation in freely-propagating laminar premixed flames, exploiting the microgravity environment to simplify measurements at the high-pressure conditions of interest for many practical applications. The findings of the investigation are relevant to reducing emissions of soot and continuum radiation from combustion processes, to improving terrestrial and spacecraft fire safety, and to developing methods of computational combustion, among others. Laminar premixed flames are attractive for studying soot formation because they are simple one-dimensional flows that are computationally tractable for detailed numerical simulations. Nevertheless, studying soot-containing burner-stabilized laminar premixed flames is problematical: spatial resolution and residence times are limited at the pressures of interest for practical applications, flame structure is sensitive to minor burner construction details so that experimental reproducibility is not very good, consistent burner behavior over the lengthy test programs needed to measure soot formation properties is hard to achieve, and burners have poor durability. Fortunately, many of these problems are mitigated for soot-containing, freely-propagating laminar premixed flames. The present investigation seeks to extend work in this laboratory for various soot processes in flames by observing soot formation in freely-propagating laminar premixed flames. Measurements are being made at both Normal Gravity (NG) and MicroGravity (MG), using a short-drop free-fall facility to provide MG conditions.

  9. Direct numerical simulation of a turbulent premixed flame

    SciTech Connect

    Hasegawa, Tatsuya; Morifuji, Tetsuya; Borghi, R.

    1999-07-01

    Direct numerical simulation of a stationary turbulent premixed flame with a single-step irreversible Arrhenius-type reaction is performed in order to understand detail physics of turbulent premixed flames and to evaluate modeling of turbulent premixed flame. The 6th-order central finite difference method is used in the streamwise direction with non-periodic boundaries, giving enough grid points in the domain to assure reasonable accuracy. The pseudo spectral method is used for transversal directions with periodic boundaries. The results obtained by their preliminary simulation is presented here with the initial turbulent intensity of u{prime}{sub 0}/u{sub L} = 4.8, the initial integral scale of l{sub t0}/{delta} = 8, and the density ratio of {rho}{sub u}/{rho}{sub b} = 7.53. The obtained flame is a developing wrinkled flame. Mean temperature, mean mass fraction, mean reaction rate and mean velocity components in space show a thickened flame region where the reaction rate appears at all points. Turbulent kinetic energy decays along the stream, but it increases somewhat in the flame region due to the increase of streamwise component of velocity fluctuation. The energy spectra in front of the flame region and behind it show that small scale decays by combustion and that the microscale and the Kolmogorov scale increase several times behind the flame region. Local structure of the turbulent flame is then analyzed.

  10. Analysis of flame surface density measurements in turbulent premixed combustion

    SciTech Connect

    Halter, Fabien; Chauveau, Christian; Goekalp, Iskender; Veynante, Denis

    2009-03-15

    In premixed turbulent combustion, reaction rates can be estimated from the flame surface density. This parameter, which measures the mean flame surface area available per unit volume, may be obtained from algebraic expressions or by solving a transport equation. In this study, detailed measurements were performed on a Bunsen-type burner fed with methane/air mixtures in order to determine the local flame surface density experimentally. This burner, located in a high-pressure combustion chamber, allows investigation of turbulent premixed flames under various flow, mixture, and pressure conditions. In the present work, equivalence ratio was varied from 0.6 to 0.8 and pressure from 0.1 to 0.9 MPa. Flame front visualizations by Mie scattering laser tomography are used to obtain experimental data on the instantaneous flame front dynamics. The exact equation given by Pope is used to obtain flame surface density maps for different flame conditions. Some assumptions are made in order to access three-dimensional information from our two-dimensional experiments. Two different methodologies are proposed and tested in term of global mass balance (what enters compared to what is burned). The detailed experimental flame surface data provided for the first time in this work should progressively allow improvement of turbulent premixed flame modeling approaches. (author)

  11. Active Control for Statistically Stationary Turbulent PremixedFlame Simulations

    SciTech Connect

    Bell, J.B.; Day, M.S.; Grcar, J.F.; Lijewski, M.J.

    2005-08-30

    The speed of propagation of a premixed turbulent flame correlates with the intensity of the turbulence encountered by the flame. One consequence of this property is that premixed flames in both laboratory experiments and practical combustors require some type of stabilization mechanism to prevent blow-off and flashback. The stabilization devices often introduce a level of geometric complexity that is prohibitive for detailed computational studies of turbulent flame dynamics. Furthermore, the stabilization introduces additional fluid mechanical complexity into the overall combustion process that can complicate the analysis of fundamental flame properties. To circumvent these difficulties we introduce a feedback control algorithm that allows us to computationally stabilize a turbulent premixed flame in a simple geometric configuration. For the simulations, we specify turbulent inflow conditions and dynamically adjust the integrated fueling rate to control the mean location of the flame in the domain. We outline the numerical procedure, and illustrate the behavior of the control algorithm on methane flames at various equivalence ratios in two dimensions. The simulation data are used to study the local variation in the speed of propagation due to flame surface curvature.

  12. Field Effects of Buoyancy on Lean Premixed Turbulent Flames

    NASA Technical Reports Server (NTRS)

    Cheng, R. K.; Johnson, M. R.; Greenberg, P. S.; Wernet, M. P.

    2003-01-01

    The study of field effects of buoyancy on premixed turbulent flames is directed towards the advancement of turbulent combustion theory and the development of cleaner combustion technologies. Turbulent combustion is considered the most important unsolved problem in combustion science and laboratory studies of turbulence flame processes are vital to theoretical development. Although buoyancy is dominant in laboratory flames, most combustion models are not yet capable to consider buoyancy effects. This inconsistency has impeded the validation of theories and numerical simulations with experiments. Conversely, the understanding of buoyancy effects is far too limited to help develop buoyant flame models. Our research is also relevant to combustion technology because lean premixed combustion is a proven method to reduce the formation of oxides of nitrogen (NOx). In industrial lean premixed combustion systems, their operating conditions make them susceptible to buoyancy thus affecting heat distribution, emissions, stability, flashback and blowoff. But little knowledge is available to guide combustion engineers as to how to avoid or overcome these problems. Our hypothesis is that through its influence on the mean pressure field, buoyancy has direct and indirect effects on local flame/turbulence interactions. Although buoyancy acts on the hot products in the farfield the effect is also felt in the nearfield region upstream of the flame. These changes also influence the generation and dissipation of turbulent kinetic energy inside the flame brush and throughout the flowfield. Moreover, the plume of an open flame is unstable and the periodic fluctuations make additional contributions to flame front dynamics in the farfield. Therefore, processes such as flame wrinkling, flow acceleration due to heat release and flame- generated vorticity are all affected. Other global flame properties (e.g. flame stabilization limits and flame speed) may all be coupled to buoyancy. This

  13. CH double-pulsed PLIF measurement in turbulent premixed flame

    NASA Astrophysics Data System (ADS)

    Tanahashi, M.; Taka, S.; Shimura, M.; Miyauchi, T.

    2008-08-01

    The flame displacement speeds in turbulent premixed flames have been measured directly by the CH double-pulsed planar laser-induced fluorescence (PLIF). The CH double-pulsed PLIF systems consist of two independent conventional CH PLIF measurement systems and laser beams from each laser system are led to same optical pass using the difference of polarization. The highly time-resolved measurements are conducted in relatively high Reynolds number turbulent premixed flames on a swirl-stabilized combustor. Since the time interval of the successive CH PLIF can be selected to any optimum value for the purpose intended, both of the large scale dynamics and local displacement of the flame front can be discussed. By selecting an appropriate time interval (100-200 μs), deformations of the flame front are captured clearly. Successive CH fluorescence images reveal the burning/generating process of the unburned mixtures or the handgrip structures in burnt gas, which have been predicted by three-dimensional direct numerical simulations of turbulent premixed flames. To evaluate the local flame displacement speed directly from the successive CH images, a flame front identification scheme and a displacement vector evaluation scheme are developed. Direct measurements of flame displacement speed are conducted by selecting a minute time interval (≈30 μs) for different Reynolds number ( Re λ = 63.1-115.0). Local flame displacement speeds coincide well for different Reynolds number cases. Furthermore, comparisons of the mean flame displacement speed and the mean fluid velocity show that the convection in the turbulent flames will affect the flame displacement speed for high Reynolds number flames.

  14. Vorticity transformation in high Karlovitz number premixed flames

    NASA Astrophysics Data System (ADS)

    Bobbitt, Brock; Lapointe, Simon; Blanquart, Guillaume

    2016-01-01

    To better understand the two-way coupling between turbulence and chemistry, the changes in turbulence characteristics through a premixed flame are investigated. Specifically, this study focuses on vorticity, ω, which is characteristic of the smallest length and time scales of turbulence, analyzing its behavior within and across high Karlovitz number (Ka) premixed flames. This is accomplished through a series of direct numerical simulations (DNS) of premixed n-heptane/air flames, modeled with a 35-species finite-rate chemical mechanism, whose conditions span a wide range of unburnt Karlovitz numbers and flame density ratios. The behavior of the terms in the enstrophy, ω2 = ω ṡ ω, transport equation is analyzed, and a scaling is proposed for each term. The resulting normalized enstrophy transport equation involves only a small set of parameters. Specifically, the theoretical analysis and DNS results support that, at high Karlovitz number, enstrophy transport obtains a balance of the viscous dissipation and production/vortex stretching terms. It is shown that, as a result, vorticity scales in the same manner as in homogeneous, isotropic turbulence within and across the flame, namely, scaling with the inverse of the Kolmogorov time scale, τη. As τη is a function only of the viscosity and dissipation rate, this work supports the validity of Kolmogorov's first similarity hypothesis in premixed turbulent flames for sufficiently high Ka numbers. Results are unaffected by the transport model, chemical model, turbulent Reynolds number, and finally the physical configuration.

  15. Premixing quality and flame stability: A theoretical and experimental study

    NASA Technical Reports Server (NTRS)

    Radhakrishnan, K.; Heywood, J. B.; Tabaczynski, R. J.

    1979-01-01

    Models for predicting flame ignition and blowout in a combustor primary zone are presented. A correlation for the blowoff velocity of premixed turbulent flames is developed using the basic quantities of turbulent flow, and the laminar flame speed. A statistical model employing a Monte Carlo calculation procedure is developed to account for nonuniformities in a combustor primary zone. An overall kinetic rate equation is used to describe the fuel oxidation process. The model is used to predict the lean ignition and blow out limits of premixed turbulent flames; the effects of mixture nonuniformity on the lean ignition limit are explored using an assumed distribution of fuel-air ratios. Data on the effects of variations in inlet temperature, reference velocity and mixture uniformity on the lean ignition and blowout limits of gaseous propane-air flames are presented.

  16. Incomplete combustion in nonadiabatic premixed gas flames

    NASA Astrophysics Data System (ADS)

    Kagan, L.; Sivashinsky, G.

    1996-06-01

    The inward propagating spherical flame and burner stabilized Bunsen-type flame of low-Lewis-number premixtures are studied numerically. It is shown that reduction of the reaction rate induced by the flame stretch makes the flame vulnerable to the radiative heat losses which may well result in a partial or complete extinction of the flame.

  17. Combustion Oscillation Analysis of Premixed Flames at Elevated Pressures

    NASA Astrophysics Data System (ADS)

    Ohtsuka, Masaya; Yoshida, Shohei; Inage, Shin'Ichi; Kobayashi, Nariyoshi

    A new analytical time lag flame model based on Bloxidge’s flame model was introduced, which calculates the combustion oscillation of premixed flame to take into account the distribution of heat release rate and flame speed that was calculated by analytical formulas dependent on pressure, temperature, fuel-to-air ratio and velocity. The transfer matrix technique using the new flame model was applied to the calculation of acoustic resonance characteristics. To verify the model, combustion oscillation experiments were performed for methane-air premixed flames stabilized by a swirl burner at elevated pressures in a range of 0.6-0.9MPa. The fluctuating pressure had a maximum peak at a specific value of fτf, where f is the resonance frequency and τf is the passing time of premixed gas through the flame zone. The analytical model could simulate the dependency of the fluctuating pressure local peak on the fuel-to-air ratio and the static pressure.

  18. Blowoff dynamics of bluff body stabilized turbulent premixed flames

    SciTech Connect

    Chaudhuri, Swetaprovo; Kostka, Stanislav; Renfro, Michael W.; Cetegen, Baki M.

    2010-04-15

    This article concerns the flame dynamics of a bluff body stabilized turbulent premixed flame as it approaches lean blowoff. Time resolved chemiluminescence imaging along with simultaneous particle image velocimetry and OH planar laser-induced fluorescence were utilized in an axisymmetric bluff body stabilized, propane-air flame to determine the sequence of events leading to blowoff and provide a quantitative analysis of the experimental results. It was found that as lean blowoff is approached by reduction of equivalence ratio, flame speed decreases and the flame shape progressively changes from a conical to a columnar shape. For a stably burning conical flame away from blowoff, the flame front envelopes the shear layer vortices. Near blowoff, the columnar flame front and shear layer vortices overlap to induce high local stretch rates that exceed the extinction stretch rates instantaneously and in the mean, resulting in local flame extinction along the shear layers. Following shear layer extinction, fresh reactants can pass through the shear layers to react within the recirculation zone with all other parts of the flame extinguished. This flame kernel within the recirculation zone may survive for a few milliseconds and can reignite the shear layers such that the entire flame is reestablished for a short period. This extinction and reignition event can happen several times before final blowoff which occurs when the flame kernel fails to reignite the shear layers and ultimately leads to total flame extinguishment. (author)

  19. Excitation of thermoacoustic oscillations by small premixed flames

    SciTech Connect

    Coats, C.M.; Chang, Z.; Williams, P.D.

    2010-06-15

    Experiments have been carried out in which very small lean premixed flames closely representative of those formed by modern multiport domestic gas burners have been subjected to controlled acoustic perturbation. PLIF from CH has been used to visualise the flame response and the heat-release-rate fluctuations have been evaluated directly from the flame images. It is shown that small laminar flames can amplify the effects of acoustic velocity fluctuations by mechanisms that do not involve resonant heat loss to the burner and that the fluctuations in flame-front area are not adequately characterised by a Strouhal number alone. The measured transfer function is compared with the predictions of various analytical formulations and a new model of the flame oscillation is proposed which applies specifically to situations in which the design of the burner renders the flame base immobile. (author)

  20. Effects of buoyancy on premixed flame stabilization

    SciTech Connect

    Bedat, B.; Cheng, R.K.

    1995-10-01

    The stabilization limits of v-flame and conical flames are investigated in normal gravity (+g) and reversed gravity (up-side-down burner, -g) to compare with observations of flame stabilization during microgravity experiments. The results show that buoyancy has most influence on the stabilization of laminar V-flames. Under turbulent conditions, the effects are less significant. For conical flames stabilized with a ring, the stabilization domain of the +g and -g cases are not significantly different. Under reversed gravity, both laminar v-flames and conical flames show flame behaviors that were also found in microgravity. The v-flames reattached to the rim and the conical flame assumed a top-hat shape. One of the special cases of -g conical flame is the buoyancy stabilized laminar flat flame that is detached from the burner. These flame implies a balance between the flow momentum and buoyant forces. The stretch rates of these flames are sufficiently low (< 20 s{sup -1}) such that the displacement speeds S{sub L} are almost equal to the laminar burning speed S{sub L}{sup 0}. An analysis based on evaluating the Richardson number is used to determine the relevant parameters that describe the buoyancy/momentum balance. A perfect balance i.e. Ri = l can be attained when the effect of heat loss from the flame zone is low. For the weaker lean cases, our assumption of adiabaticity tends to overestimate the real flame temperature. This interesting low stretch laminar flame configuration can be useful for fundamental studies of combustion chemistry.

  1. Characteristics of Non-Premixed Turbulent Flames in Microgravity

    NASA Technical Reports Server (NTRS)

    Hegde, U.; Yuan, Z. G.; Stocker, D. P.; Bahadori, M. Y.

    2001-01-01

    This project is concerned with the characteristics of turbulent hydrocarbon (primarily propane) gas-jet diffusion flames in microgravity. A microgravity environment provides the opportunity to study the structure of turbulent diffusion flames under momentum-dominated conditions (large Froude number) at moderate Reynolds number which is a combination not achievable in normal gravity. This paper summarizes progress made since the last workshop. Primarily, the features of flame radiation from microgravity turbulent jet diffusion flames in a reduced gravity environment are described. Tests were conducted for non-premixed, nitrogen diluted propane flames burning in quiescent air in the NASA Glenn 5.18 Second Zero Gravity Facility. Measured flame radiation from wedge-shaped, axial slices of the flame are compared for microgravity and normal gravity flames. Results from numerical computations of the flame using a k-e model for the turbulence are also presented to show the effects of flame radiation on the thermal field. Flame radiation is an important quantity that is impacted by buoyancy as has been shown in previous studies by the authors and also by Urban et al. It was found that jet diffusion flames burning under microgravity conditions have significantly higher radiative loss (about five to seven times higher) compared to their normal gravity counterparts because of larger flame size in microgravity and larger convective heat loss fraction from the flame in normal gravity. These studies, however, were confined to laminar flames. For the case of turbulent flames, the flame radiation is a function of time and both the time-averaged and time-dependent components are of interest. In this paper, attention is focused primarily on the time-averaged level of the radiation but the turbulent structure of the flame is also assessed from considerations of the radiation power spectra.

  2. Partially premixed flames in stagnating turbulence: The merging of planar triple flames

    SciTech Connect

    Bray, Ken; Champion, Michel; Libby, Paul A.

    2008-07-15

    The aim of this work, which takes a RANS perspective, is to consider the prospect of establishing a planar turbulent triple flame whose mean consists of two parallel premixed flame brushes separated by a nonpremixed flame brush. Experiments involving a counterflow between fuel-rich and fuel-lean turbulent streams are considered. A correlation of published experimental data is used to estimate premixed turbulent flame brush locations and brush thicknesses. Previously validated model calculations then allow an estimate to be made of the thickness of a central nonpremixed flame or mixing layer, a thickness which is shown to be strongly influenced by flame-turbulence interactions in the premixed flames. This thickness turns out to be orders-of-magnitude greater than the width of the hot burned gas region between the two premixed flames strongly suggesting that the three reacting flow regions will merge with each other. It is concluded that unlike the corresponding laminar counterflow planar turbulent triple flames will be difficult to establish in laboratory scale experiments. (author)

  3. Some effects of heat release in premixed flames

    SciTech Connect

    Shepherd, I.G.

    1994-03-01

    Numerical and experimental results are presented to illustrate some hydrodynamic effects of heat release in premixed flames. The heat release is represented by a simple model which treats the flame front as a two dimensional line source of volume. The velocity and strain rate induced in the flow field are determined and the numerical solution for the case of a laminar double kernel ignition is obtained. Of primary interest is the strain induced in the reactants between the expanding flame kernels and, for heat release rates typical of hydrocarbon flames, the strain rate at the plane of symmetry midway between the kernels up to 150 s{sup {minus}1}. The effects of kernel size, density ratio across the flame front and laminar burning velocity are studied. For the case of turbulent combustion the velocity induced in the reactant stream is measured in a plane parallel to the flame holder of an open premixed turbulent V-shaped flame. A divergent flow field, with a strain rate of 50 s{sup {minus}1}, is induced by the heat release in the flame zone and the consequences of this for determining the turbulent burning velocity in this and similar systems is reviewed.

  4. Accelerative propagation and explosion triggering by expanding turbulent premixed flames.

    PubMed

    Akkerman, V'yacheslav; Chaudhuri, Swetaprovo; Law, Chung K

    2013-02-01

    The dynamics and morphology of outwardly propagating, accelerating turbulent premixed flames and the effect of flame acceleration on explosion triggering are analyzed. Guided by recent theoretical results and substantiated by experiments, we find that an expanding flame front in an externally forced, near-isotropic turbulent environment exhibits accelerative propagation given by a well-defined power law based on the average global flame radius. In this context the limits of the power-law exponent and the effective turbulence intensity experienced by the flame are derived. The power-law exponent is found to be substantially larger than that for the hydrodynamically unstable cellular laminar flames, hence facilitating the possibility of detonation triggering in turbulent environments. For large length scales, hydrodynamic instability is expected to provide additional acceleration, thus further favoring the attainment of detonation triggering.

  5. Dynamics of premixed hydrogen/air flames in mesoscale channels

    SciTech Connect

    Pizza, Gianmarco; Frouzakis, Christos E.; Boulouchos, Konstantinos; Mantzaras, John; Tomboulides, Ananias G.

    2008-10-15

    Direct numerical simulation with detailed chemistry and transport is used to study the stabilization and dynamics of lean ({phi}=0.5) premixed hydrogen/air atmospheric pressure flames in mesoscale planar channels. Channel heights of h=2, 4, and 7 mm, and inflow velocities in the range 0.3{<=}U{sub IN}{<=}1100cm/ s are investigated. Six different burning modes are identified: mild combustion, ignition/extinction, closed steady symmetric flames, open steady symmetric flames, oscillating and, finally, asymmetric flames. Chaotic behavior of cellular flame structures is observed for certain values of U{sub IN}. Stability maps delineating the regions of the different flame types are finally constructed. (author)

  6. Partially Premixed Flame (PPF) Research for Fire Safety

    NASA Technical Reports Server (NTRS)

    Puri, Ishwar K.; Aggarwal, Suresh K.; Lock, Andrew J.; Hegde, Uday

    2004-01-01

    Incipient fires typically occur after the partial premixing of fuel and oxidizer. The mixing of product species into the fuel/oxidizer mixture influences flame stabilization and fire spread. Therefore, it is important to characterize the impact of different levels of fuel/oxidizer/product mixing on flame stabilization, liftoff and extinguishment under different gravity conditions. With regard to fire protection, the agent concentration required to achieve flame suppression is an important consideration. The initial stage of an unwanted fire in a microgravity environment will depend on the level of partial premixing and the local conditions such as air currents generated by the fire itself and any forced ventilation (that influence agent and product mixing into the fire). The motivation of our investigation is to characterize these impacts in a systematic and fundamental manner.

  7. Freely propagating open premixed turbulent flames stabilized by swirl

    SciTech Connect

    Chan, C.K.; Lau, K.S.; Chin, W.K.; Cheng, R.K.

    1991-12-01

    A novel means has been developed for using weak swirl to stabilize freely propagating open premixed turbulent flames (swirl numbers between 0.05 to 0.3). By injecting a small amount of air tangentially into the co-flow of a concentric burner, stationary flames can be maintained above the burner exit for a large range of mixture, turbulence and flow conditions. The absence of physical surfaces in the vicinity of the flame provides free access to laser diagnostics. Laser Doppler anemometry and laser Mie scattering measurements of four flames with and without incident turbulence show that their features are typical of wrinkled laminar flames. The most distinct characteristics is that flame stabilization does not rely on flow recirculation. Centrifugal force induced by swirl causes flow divergence, and the flame is maintained at where the local mass flux balances the burning rate. The flame speeds can be estimated based on the centerline velocity vector, which is locally normal to the flame brush. This flame geometry is the closest approximation to the 1-D planar flame for determining fundamental properties to advance turbulent combustion theories. 18 refs.

  8. An evaluation of different contributions to flame stretch for stationary premixed flames

    SciTech Connect

    Goey, L.P.H. de; Mallens, R.M.M.; Thije Boonkkamp, J.H.M. ten

    1997-07-01

    The concept of flame stretch is extended to study stationary premixed flames with a finite thickness. It is shown that the analysis results in additional contributions to the stretch rate due to changes in the flame thickness and due to density variations along the flame. Extended expressions are derived that describe the effect of stretch on variations in scalar quantities, such as the enthalpy. These expressions are used to determine local variations in the flame temperature, and it is shown that known results are recovered when a number of approximations are introduced. The extended stretch formalism might be useful to analyze and quantify the different flame stretch contributions and their effects in numerical flame studies. Finally, the different contributions to the total stretch rate and the effects thereof on the flame stabilization are numerically computed for the flame tip of a two-dimensional Bunsen flame as illustration.

  9. Streamline segment statistics of premixed flames with nonunity Lewis numbers

    NASA Astrophysics Data System (ADS)

    Chakraborty, Nilanjan; Wang, Lipo; Klein, Markus

    2014-03-01

    The interaction of flame and surrounding fluid motion is of central importance in the fundamental understanding of turbulent combustion. It is demonstrated here that this interaction can be represented using streamline segment analysis, which was previously applied in nonreactive turbulence. The present work focuses on the effects of the global Lewis number (Le) on streamline segment statistics in premixed flames in the thin-reaction-zones regime. A direct numerical simulation database of freely propagating thin-reaction-zones regime flames with Le ranging from 0.34 to 1.2 is used to demonstrate that Le has significant influences on the characteristic features of the streamline segment, such as the curve length, the difference in the velocity magnitude at two extremal points, and their correlations with the local flame curvature. The strengthenings of the dilatation rate, flame normal acceleration, and flame-generated turbulence with decreasing Le are principally responsible for these observed effects. An expression for the probability density function (pdf) of the streamline segment length, originally developed for nonreacting turbulent flows, captures the qualitative behavior for turbulent premixed flames in the thin-reaction-zones regime for a wide range of Le values. The joint pdfs between the streamline length and the difference in the velocity magnitude at two extremal points for both unweighted and density-weighted velocity vectors are analyzed and compared. Detailed explanations are provided for the observed differences in the topological behaviors of the streamline segment in response to the global Le.

  10. Extinction conditions of a premixed flame in a channel

    SciTech Connect

    Alliche, Mounir; Haldenwang, Pierre; Chikh, Salah

    2010-06-15

    A local refinement method is used to numerically predict the propagation and extinction conditions of a premixed flame in a channel considering a thermodiffusive model. A local refinement method is employed because of the numerous length scales that characterize this phenomenon. The time integration is self adaptive and the solution is based on a multigrid method using a zonal mesh refinement in the flame reaction zone. The objective is to determine the conditions of extinction which are characterized by the flame structure and its properties. We are interested in the following properties: the curvature of the flame, its maximum temperature, its speed of propagation and the distance separating the flame from the wall. We analyze the influence of heat losses at the wall through the thermal conductivity of the wall and the nature of the fuel characterized by the Lewis number of the mixture. This investigation allows us to identify three propagation regimes according to heat losses at the wall and to the channel radius. The results show that there is an intermediate value of the radius for which the flame can bend and propagate provided that its curvature does not exceed a certain limit value. Indeed, small values of the radius will choke the flame and extinguish it. The extinction occurs if the flame curvature becomes too small. Furthermore, this study allows us to predict the limiting values of the heat loss coefficient at extinction as well as the critical value of the channel radius above which the premixed flame may propagate without extinction. A dead zone of length 2-4 times the flame thickness appears between the flame and the wall for a Lewis number (Le) between 0.8 and 2. For small values of Le, local extinctions are observed. (author)

  11. Behaviour of a Premixed Flame Subjected to Acoustic Oscillations

    PubMed Central

    Qureshi, Shafiq R.; Khan, Waqar A.; Prosser, Robert

    2013-01-01

    In this paper, a one dimensional premixed laminar methane flame is subjected to acoustic oscillations and studied. The purpose of this analysis is to investigate the effects of acoustic perturbations on the reaction rates of different species, with a view to their respective contribution to thermoacoustic instabilities. Acoustically transparent non reflecting boundary conditions are employed. The flame response has been studied with acoustic waves of different frequencies and amplitudes. The integral values of the reaction rates, the burning velocities and the heat release of the acoustically perturbed flame are compared with the unperturbed case. We found that the flame's sensitivity to acoustic perturbations is greatest when the wavelength is comparable to the flame thickness. Even in this case, the perturbations are stable with time. We conclude that acoustic fields acting on the chemistry do not contribute significantly to the emergence of large amplitude pressure oscillations. PMID:24376501

  12. Stabilization of premixed flames on rotating Bunsen burners

    SciTech Connect

    Cha, J.M.; Sohrab, S.H.

    1996-09-01

    The effect of rotation on stabilization of methane-air premixed Bunsen flame sis experimentally investigated. Both the flame blowoff and flashback contours are determined in the fuel mole fraction versus Reynolds number plane (X{sub F}-Re) with the rotational Reynolds number Re{sub 4} as a parameter. It is found that rotation of the gas increases the flame stabilization area A{sub s} = A{sub B} {minus} A{sub F} defined as the difference between the flame blowoff A{sub B} and flashback A{sub F} areas in the (X{sub F}-Re) plane. The flame stabilization efficiency is defined as {eta}{sub s} = 1 {minus} A{sub F}/A{sub B} that approaches unity in either A{sub B} {yields} {infinity} or A{sub F} {yields} 0 limit. The experimental results suggest that rotation decreases the flame stabilization efficiency. However, rotation is found to substantially increase the flame stabilization coefficient defined as {beta}{sub s} = A{sub s}/A{sub st}, where A{sub st} is the stabilization area of the standard nonrotating burner. The parameters {eta}{sub s} and {beta}{sub s} may be useful in combustion technology for quantitative evaluation of the stabilization performance of different types of flame holders. In addition, the local hydrodynamics near the center of rotating Bunsen burner is simulated by investigating stabilization of planar laminar premixed flames on rotating porous disks with uniform surface velocity. Physical concepts concerning mechanisms of flame stabilization are discussed in terms of three important parameters namely the translational Reynolds number Re, the rotation Reynolds number Re{sub r}, and the fuel mole fraction X{sub F}. The results of the experimental findings are shown to be in accordance with prior theoretical investigation.

  13. Vorticity isotropy in high Karlovitz number premixed flames

    NASA Astrophysics Data System (ADS)

    Bobbitt, Brock; Blanquart, Guillaume

    2016-10-01

    The isotropy of the smallest turbulent scales is investigated in premixed turbulent combustion by analyzing the vorticity vector in a series of high Karlovitz number premixed flame direct numerical simulations. It is found that increasing the Karlovitz number and the ratio of the integral length scale to the flame thickness both reduce the level of anisotropy. By analyzing the vorticity transport equation, it is determined that the vortex stretching term is primarily responsible for the development of any anisotropy. The local dynamics of the vortex stretching term and vorticity resemble that of homogeneous isotropic turbulence to a greater extent at higher Karlovitz numbers. This results in small scale isotropy at sufficiently high Karlovitz numbers and supports a fundamental similarity of the behavior of the smallest turbulent scales throughout the flame and in homogeneous isotropic turbulence. At lower Karlovitz numbers, the vortex stretching term and the vorticity alignment in the strain-rate tensor eigenframe are altered by the flame. The integral length scale has minimal impact on these local dynamics but promotes the effects of the flame to be equal in all directions. The resulting isotropy in vorticity does not reflect a fundamental similarity between the smallest turbulent scales in the flame and in homogeneous isotropic turbulence.

  14. Response mechanisms of attached premixed flames subjected to harmonic forcing

    NASA Astrophysics Data System (ADS)

    Shreekrishna

    The persistent thrust for a cleaner, greener environment has prompted air pollution regulations to be enforced with increased stringency by environmental protection bodies all over the world. This has prompted gas turbine manufacturers to move from nonpremixed combustion to lean, premixed combustion. These lean premixed combustors operate quite fuel-lean compared to the stochiometric, in order to minimize CO and NOx productions, and are very susceptible to oscillations in any of the upstream flow variables. These oscillations cause the heat release rate of the flame to oscillate, which can engage one or more acoustic modes of the combustor or gas turbine components, and under certain conditions, lead to limit cycle oscillations. This phenomenon, called thermoacoustic instabilities, is characterized by very high pressure oscillations and increased heat fluxes at system walls, and can cause significant problems in the routine operability of these combustors, not to mention the occasional hardware damages that could occur, all of which cumulatively cost several millions of dollars. In a bid towards understanding this flow-flame interaction, this research works studies the heat release response of premixed flames to oscillations in reactant equivalence ratio, reactant velocity and pressure, under conditions where the flame preheat zone is convectively compact to these disturbances, using the G-equation. The heat release response is quantified by means of the flame transfer function and together with combustor acoustics, forms a critical component of the analytical models that can predict combustor dynamics. To this end, low excitation amplitude (linear) and high excitation amplitude (nonlinear) responses of the flame are studied in this work. The linear heat release response of lean, premixed flames are seen to be dominated by responses to velocity and equivalence ratio fluctuations at low frequencies, and to pressure fluctuations at high frequencies which are in the

  15. Measurements of turbulent premixed flame dynamics using cinema stereoscopic PIV

    NASA Astrophysics Data System (ADS)

    Steinberg, Adam M.; Driscoll, James F.; Ceccio, Steven L.

    2008-06-01

    A new experimental method is described that provides high-speed movies of turbulent premixed flame wrinkling dynamics and the associated vorticity fields. This method employs cinema stereoscopic particle image velocimetry and has been applied to a turbulent slot Bunsen flame. Three-component velocity fields were measured with high temporal and spatial resolutions of 0.9 ms and 140 μm, respectively. The flame-front location was determined using a new multi-step method based on particle image gradients, which is described. Comparisons are made between flame fronts found with this method and simultaneous CH-PLIF images. These show that the flame contour determined corresponds well to the true location of maximum gas density gradient. Time histories of typical eddy-flame interactions are reported and several important phenomena identified. Outwardly rotating eddy pairs wrinkle the flame and are attenuated at they pass through the flamelet. Significant flame-generated vorticity is produced downstream of the wrinkled tip. Similar wrinkles are caused by larger groups of outwardly rotating eddies. Inwardly rotating pairs cause significant convex wrinkles that grow as the flame propagates. These wrinkles encounter other eddies that alter their behavior. The effects of the hydrodynamic and diffusive instabilities are observed and found to be significant contributors to the formation and propagation of wrinkles.

  16. The propagation of premixed flames in closed tubes

    NASA Astrophysics Data System (ADS)

    Matalon, Moshe; Metzener, Philippe

    1997-04-01

    A nonlinear evolution equation that describes the propagation of a premixed flame in a closed tube has been derived from the general conservation equations. What distinguishes it from other similar equations is a memory term whose origin is in the vorticity production at the flame front. The two important parameters in this equation are the tube's aspect ratio and the Markstein parameter. A linear stability analysis indicates that when the Markstein parameter [alpha] is above a critical value [alpha]c the planar flame is the stable equilibrium solution. For [alpha] below [alpha]c the planar flame is no longer stable and there is a band of growing modes. Numerical solutions of the full nonlinear equation confirm this conclusion. Starting with random initial conditions the results indicate that, after a short transient, a at flame develops when [alpha]>[alpha]c and it remains flat until it reaches the end of the tube. When [alpha]<[alpha]c, on the other hand, stable curved flames may develop down the tube. Depending on the initial conditions the flame assumes either a cellular structure, characterized by a finite number of cells convex towards the unburned gas, or a tulip shape characterized by a sharp indentation at the centre of the tube pointing toward the burned gases. In particular, if the initial conditions are chosen so as to simulate the elongated finger-like flame that evolves from an ignition source, a tulip flame evolves downstream. In accord with experimental observations the tulip shape forms only after the flame has travelled a certain distance down the tube, it does not form in short tubes and its formation depends on the mixture composition. While the initial deformation of the flame front is a direct result of the hydrodynamic instability, the actual formation of the tulip flame results from the vortical motion created in the burned gas which is a consequence of the vorticity produced at the flame front.

  17. Premixed silane-oxygen-nitrogen flames

    SciTech Connect

    Tokuhashi, K.; Horiguchi, S.; Uranco, Y.; Iwasaka, M.; Ohtani, H.; Kondo, S. )

    1990-10-01

    The burning velocities of lean premised silane-oxygen-nitrogen flames were measured in the silane and oxygen concentration ranges from 1.6% to 2.9% and from 4% to 24%, respectively. Combustion product analyses and flame temperature measurements were also carried out. The burning velocity of a silane-air flame is around 55 cm/ at a silane concentration of 2%. For lean mixtures, when the oxygen concentration is reduced, dependence of burning velocity upon silane concentration decreases but does not significantly affect the flame temperature. For extremely lean flames, the degree of hydrogen production increase with decreasing silane, although silane is consumed almost completely. On the other hand, if the silane concentration exceeds stoichiometric, the burning velocity increases gradually with increasing silane concentration. In that case, silane as well as oxygen are consumed completely and, at the same time, hydrogen rather than water production becomes dominant. The mechanism of silane combustion is discussed, based on numerical calculations, where the mechanism used in the calculation is assembled by analogy of silane to methane combustion.

  18. Stationary premixed flames in spherical and cylindrical geometries

    NASA Technical Reports Server (NTRS)

    Ronney, P. D.; Whaling, K. N.; Abbud-Madrid, A.; Gatto, J. L.; Pisowiscz, V. L.

    1994-01-01

    Stationary source-free spherical flames ('flame balls') in premixed combustible gases were studied by employing low-gravity (micro-g) environments in a drop tower and an aircraft flying parabolic trajectories to diminish the impact of buoyancy-induced convective flow. Flame balls were found in all mixture families tested when: (1) the Lewis number Le of the deficient reactant was sufficiently low; and (2) the compositions were sufficiently close to the flammability limits. Probably as a consequence of the reduction in buoyant convection, the flammability limits at micro-g were significantly more dilute than those at Earth gravity; for example, 3.35% H2 vs 4.0% H2 in lean H2-air mixtures. By comparison with analytical and computational models, it is inferred that the phenomenon is probably related to diffusive-thermal effects in low-Le mixtures in conjunction with flame-front curvature and radiative heat losses from the combustion products. The chemical reaction mechanism appears to play no qualitative role. In the aircraft experiments, the gravity levels (approximately equal 10(exp -2)g(sub 0)) were found to cause noticeable motion of flame balls due to buoyancy, which in turn influenced the behavior of flame balls. At these g levels, a new type of transient, nearly cylindrical flame structure, termed 'flame strings,' was observed.

  19. Non-premixed acoustically perturbed swirling flame dynamics

    SciTech Connect

    Idahosa, Uyi; Saha, Abhishek; Xu, Chengying; Basu, Saptarshi

    2010-09-15

    An investigation into the response of non-premixed swirling flames to acoustic perturbations at various frequencies (f{sub p}=0-315 Hz) and swirl intensities (S=0.09 and 0.34) is carried out. Perturbations are generated using a loudspeaker at the base of an atmospheric co-flow burner with resulting velocity oscillation amplitudes vertical stroke u'/U{sub avg} vertical stroke in the 0.03-0.30 range. The dependence of flame dynamics on the relative richness of the flame is investigated by studying various constant fuel flow rate flame configurations. Flame heat release rate is quantitatively measured using a photomultiplier with a 430 nm bandpass filter for observing CH* chemiluminescence which is simultaneously imaged with a phase-locked CCD camera. The flame response is observed to exhibit a low-pass filter characteristic with minimal flame response beyond pulsing frequencies of 200 Hz. Flames at lower fuel flow rates are observed to remain attached to the central fuel pipe at all acoustic pulsing frequencies. PIV imaging of the associated isothermal fields show the amplification in flame aspect ratio is caused by the narrowing of the inner recirculation zone (IRZ). Good correlation is observed between the estimated flame surface area and the heat release rate signature at higher swirl intensity flame configurations. A flame response index analogous to the Rayleigh criterion in non-forced flames is used to assess the potential for a strong flame response at specific perturbation configurations and is found to be a good predictor of highly responsive modes. Phase conditioned analysis of the flame dynamics yield additional criteria in highly responsive modes to include the effective amplitude of velocity oscillations induced by the acoustic pulsing. In addition, highly responsive modes were characterized by velocity to heat release rate phase differences in the {+-}{pi}/2 range. A final observed characteristic in highly responsive flames is a Strouhal number between

  20. Flame Oscillations In Non-Premixed Systems Diffusion Flames and Edge-Flames

    NASA Technical Reports Server (NTRS)

    Matalon, Moshe

    2003-01-01

    Diffusive-thermal instabilities are well known features of premixed and diffusion flames. In one of its form the instability appears as spontaneous oscillations. In premixed systems oscillations are predicted to occur when the effective Lewis number, defined as the ratio of the thermal diffusivity of the mixture to the mass diffusivity of the deficient component, is sufficiently larger than one. Oscillations would therefore occur in mixtures that are deficient in the less mobile reactant, namely in lean hydrocarbon-air or rich hydrogen-air mixtures. The theoretical predictions summarized above are in general agreement with experimental results; see for example [5] where a jet configuration was used and experiments were conducted for various inert-diluted propane and methane flames burning in inert-diluted oxygen. Nitrogen, argon and SF6 were used as inert in order to produce conditions of substantially different Lewis numbers and mixture strength. In accord with the predicted trend, it was found that oscillations arise at near extinction conditions, that for oscillations to occur it suffices that one of the two Lewis numbers be sufficiently large, and that oscillations are more likely to be observed when is relatively large.

  1. Premixed burner experiments: Geometry, mixing, and flame structure issues

    SciTech Connect

    Gupta, A.K.; Lewis, M.J.; Gupta, M.

    1995-10-01

    This research program is exploring techniques for improved fuel-air mixing, with the aim of achieving combustor operations up to stoichiometric conditions with minimal NO x and maximum efficiency. The experimental studies involve the use of a double-concentric natural gas burner that is operable in either premixed or non-premixed modes, and the system allows systematic variation of equivalence ratio, swirl strength shear length region and flow momentum in each annulus. Flame structures formed with various combinations of swirl strengths, flow throughput and equivalence ratios in premixed mode show the significant impact of swirl flow distribution on flame structure emanating from the mixedness. This impact on flame structure is expected to have a pronounced effect on the heat release rate and the emission of NO{sub x}. Thus, swirler design and configuration remains a key factor in the quest for completely optimized combustion. Parallel numerical studies of the flow and combustion phenomena were carried out, using the RSM and thek-{epsilon} turbulence models. These results have not only indicated the strengths and limitations of CFD in performance and pollutants emission predictions, but have provided guidelines on the size and strength of the recirculation produced and the spatio-temporal structure of the combustion flowfield. The first stage of parametric studies on geometry and operational parameters at Morgan State University have culminated in the completion of a one-dimensional flow code that is integrated with a solid, virtual model of the existing premixed burner. This coupling will provide the unique opportunity to study the impact of geometry on the flowfield and vice-versa, with particular emphasis on concurrent design optimization.

  2. A ring stabilizer for lean premixed turbulent flames

    SciTech Connect

    Johnson, M.R.; Kostiuk, L.W.; Cheng, R.K.

    1998-08-01

    In previous experiments on conical flame behavior in microgravity, which were conducted in drop-towers and in airplanes, the use of a pilot flame was not an option. To permit combustion of stable lean premixed conical flames without a pilot, a ring stabilizer was developed. Although similar types of bluff-body stabilization have been used in the past, the ring stabilizer is somewhat unique. It is designed to fit inside the burner exit port and has demonstrated to be highly effective in stabilizing flames over a very wide range of conditions (including ultra-lean flames at high flow-rates) without adversely affecting flame emissions. Unlike a simple rod stabilizer or a stagnation flame system, the benefit of having the stabilizer conform to the burner port is that there is very little leakage of the unburned fuel. The purpose of this brief communication is to offer this simple and highly useful device to the combustion research community. Presented are highlights of a parametric study that measured the stabilization limits and pollutant emissions of several different rings, and demonstrated their potential for use in practical systems.

  3. Stability Enhancement of Lean, Premixed Flames by Flameholder Heating

    NASA Astrophysics Data System (ADS)

    Hermanson, James C.; Demmons, Nathaniel

    2001-11-01

    The effects of flameholder heating on the stability and emissions of lean, premixed, turbulent flames were examined experimentally. The flames were stabilized by an axial, cylindrical bluff-body flameholder 6.4 mm in diameter made of copper or stainless steel. In some cases, the stainless flameholder was heated electrically. The flame was at atmospheric pressure. The premixed ethylene/air mixture upstream of the flameholder was unheated and had an equivalence ratio of 0.37 to 0.87. The cold gas flow velocities ranged from 5.0 to 10.5 m/s to give Reynolds numbers at the flameholder tip from 3,250 to 6,700. The impact of flameholder heating on the lean-blow off limit was determined visually. Heating the flameholder to yield a local mixture temperature of 190 C resulted in a decrease in the equivalence ratio at lean blow-off of approximately 20%. This decrease in equivalence ratio resulted in up to a 26% decrease in exhaust-plane NOx emissions and a 51 K reduction in the exhaust-plane gas temperature. These reductions were consistent with the lower equivalence ratios attainable by the localized mixture preheating. At the same time, the exhaust concentrations of CO and unburned hydrocarbons increased by a factor of approximately two. A smaller increase in lean flame stability was seen for the unheated stainless flameholder versus the copper flameholder.

  4. Preflame zone structure and main features of fuel conversion in atmospheric pressure premixed laminar hydrocarbon flames

    SciTech Connect

    Ksandopulo, G.I.

    1995-08-25

    This report describes the structure study of the premixed hydrocarbon-oxidizer Bunsen flames burning at the atmospheric pressure and also the ones with some inhibitors added. Studies were performed on hexane, propane, methane, acetylene, and hexene flames.

  5. An experimental investigation of an acoustically excited laminar premixed flame

    SciTech Connect

    Kartheekeyan, S.; Chakravarthy, S.R.

    2006-08-15

    A two-dimensional laminar premixed flame is stabilized over a burner in a confined duct and is subjected to external acoustic forcing from the downstream end. The equivalence ratio of the flame is 0.7. The flame is stabilized in the central slot of a three-slotted burner. The strength of the shear layer of the cold reactive mixture through the central slot is controlled by the flow rate of cold nitrogen gas through the side slots. The frequency range of acoustic excitation is 400-1200 Hz, and the amplitude levels are such that the acoustic velocity is less than the mean flow velocity of the reactants. Time-averaged chemiluminescence images of the perturbed flame front display time-mean changes as compared to the unperturbed flame shape at certain excitation frequencies. Prominent changes to the flame front are in the form of stretching or shrinkage, asymmetric development of its shape, increased/preferential lift-off of one or both of the stabilization points of the flame, and nearly random three-dimensional fluctuations over large time scales under some conditions. The oscillations of the shear layer and the response of the confined jet of the hot products to the acoustic forcing, such as asymmetric flow development and jet spreading, are found to be responsible for the observed mean changes in the flame shape. A distinct low-frequency component ({approx}60-90 Hz) relative to the excitation frequency is observed in the fluctuations of the chemiluminescent intensity in the flame under most conditions. It is observed that fluctuations in the flame area predominantly contribute to the origin of the low-frequency component. This is primarily due to the rollup of vortices and the generation of enthalpy waves at the burner lip. Both of these processes are excited at the externally imposed acoustic time scale, but convect/propagate downstream at the flow time scale, which is much larger. (author)

  6. Bifurcation characteristics and flame dynamics of a ducted non-premixed flame with finite rate chemistry

    NASA Astrophysics Data System (ADS)

    Rana, Subhas Chandra; Sujith, Raman

    2015-09-01

    The influence of system parameters such as the flame location, Peclet number and Damköhler number on the bifurcation characteristics and flame dynamics of a ducted non-premixed flame with finite rate chemistry is presented in this paper. In the bifurcation plot with flame location as the bifurcation parameter, subcritical Hopf bifurcation is found for lower values of flame location and supercritical Hopf bifurcation for higher values of flame location, for all the Damköhler numbers used in this study. The flame shapes are captured at eight different phases of a cycle of time series data of acoustic velocity at both the fold and Hopf points for bifurcation with flame location as the parameter. We find that the range of flame height variations at the Hopf point is more than the range of flame height variations obtained at the fold point. We also find that the flame oscillates in the same phase as pressure fluctuation but in a phase different from both velocity and heat release rate fluctuations in the region of hysteresis for bifurcation with flame location. The non-dimensional hysteresis width is plotted as a function of Damköhler number for variation of flame location in the subcritical region. An inverse power law relation is found between the non-dimensional hysteresis width and the Damköhler number. The bifurcation plot with Peclet number as parameter shows a subcritical Hopf bifurcation.

  7. Premixed-Gas Flame Propagation in Hele-Shaw Cells

    NASA Technical Reports Server (NTRS)

    Sharif, J.; Abid, M.; Ronney, P. D.

    1999-01-01

    It is well known that buoyancy and thermal expansion affect the propagation ra and shapes of premixed gas flames. The understanding of such effects is complicated by the large density ratio between the reactants and products, which induces a baroclinic production of vorticity due to misalignment of density and pressure gradients at the front, which in turn leads to a complicated multi-dimensional flame/flow interaction. The Hele-Shaw cell, i.e., the region between closely-spaced flat parallel plates, is probably the simplest system in which multi-dimensional convection is presents consequently, the behavior of fluids in this system has been studied extensively (Homsy, 1987). Probably the most important characteristic of Hele-Shaw flows is that when the Reynolds number based on gap width is sufficiently small, the Navier-Stokes equations averaged over the gap reduce to a linear relation, namely a Laplace equation for pressure (Darcy's law). In this work, flame propagation in Hele-Shaw cells is studied to obtain a better understanding of buoyancy and thermal expansion effects on premixed flames. This work is also relevant to the study of unburned hydrocarbon emissions produced by internal combustion engines since these emissions are largely a result of the partial burning or complete flame quenching in the narrow, annular gap called the "crevice volume" between the piston and cylinder walls (Heywood, 1988). A better understanding of how flames propagate in these volumes through experiments using Hele-Shaw cells could lead to identification of means to reduce these emissions.

  8. Transport of inertial particles in a turbulent premixed jet flame

    NASA Astrophysics Data System (ADS)

    Battista, F.; Picano, F.; Troiani, G.; Casciola, C. M.

    2011-12-01

    The heat release, occurring in reacting flows, induces a sudden fluid acceleration which particles follow with a certain lag, due to their finite inertia. Actually, the coupling between particle inertia and the flame front expansion strongly biases the spatial distribution of the particles, by inducing the formation of localized clouds with different dimensions downstream the thin flame front. A possible indicator of this preferential localization is the so-called Clustering Index, quantifying the departure of the actual particle distribution from the Poissonian, which would correspond to a purely random spatial arrangement. Most of the clustering is found in the flame brush region, which is spanned by the fluctuating instantaneous flame front. The effect is significant also for very light particles. In this case a simple model based on the Bray-Moss-Libby formalism is able to account for most of the deviation from the Poissonian. When the particle inertia increases, the effect is found to increases and persist well within the region of burned gases. The effect is maximum when the particle relaxation time is of the order of the flame front time scale. The evidence of this peculiar source of clustering is here provided by data from a direct numerical simulation of a turbulent premixed jet flame and confirmed by experimental data.

  9. A high-pressure premixed flat-flame burner for chemical process studies. [of pollutant formation in hydrocarbon flames

    NASA Technical Reports Server (NTRS)

    Miller, I. M.

    1978-01-01

    A premixed flat-flame burner was designed and tested with methane-air mixtures at pressures from 1.1 to 20 atm and equivalence ratios from 0.7 to 1.1. Reactant velocity in the burner mixing chamber was used to characterize the range of stable flames at each pressure-equivalence-ratio condition. Color photographs of the flames were used to determine flame zone thickness and flame height. The results show that this burner can be used for chemical process studies in premixed high pressure methane-air flames up to 20 atm.

  10. Simulation of flame surface density and burning rate of a premixed turbulent flame using contour advection

    SciTech Connect

    Tang, B.H.Y.; Chan, C.K.

    2006-10-15

    In this paper, a 2-dimensional rod-stabilized V-shaped flame is simulated using contour advection with surgery as well as the random vortex method. Effects of turbulence on various quantities, such as flame brush thickness and flame surface density, are investigated. The flame surface density S is estimated using the Bray-Moss-Libby formulation, which involves the use of a mean orientation factor {sigma}{sub c}. As a comparison, values of S are also obtained using Shepherd's model, which employs the values of mean flame surface area and mean flame length. Local flame structure is characterized in terms of turbulent flame brush, orientation factor, and flame surface density. Profiles of S obtained using the two different models are compared and show that discrepancy is more evident with increasing turbulence intensity. (author)

  11. Lean premixed flames for low NO{sub x} combustors

    SciTech Connect

    Sojka, P.; Tseng, L.; Bryyjak, J.

    1995-12-31

    The overall objectives of the research at Purdue are to: obtain a reduced mechanism description of high pressure NO formation chemistry using experiments and calculations for laminar lean premixed methane air flames, develop a statistical model of turbulence NO chemistry interactions using a Bunsen type jet flame, and utilize the high pressure chemistry and turbulence models in a commercial design code, then evaluate its predictions using data from an analog gas turbine combustor. Work to date has resulted in the following achievements: spatially resolved measurements of NO in high-pressure high-temperature flat flames, plus evaluation of the influence of flame radiation on the measured temperature profile; measurements of temperature and velocity PDFs for a turbulent methane/air flame were obtained for the first time, under operating conditions which allow their study in the distributed regimes, and the increase in EINO{sub x} with equivalence ratio predicted using a chemical kinetics model; and simulation of non-reacting combustor flow fields from ambient to elevated pressure and temperature conditions and comparison of those results with experimental velocity profiles.

  12. Numerical simulation of premixed flame propagation in a closed tube

    NASA Astrophysics Data System (ADS)

    Kuzuu, Kazuto; Ishii, Katsuya; Kuwahara, Kunio

    1996-08-01

    Premixed flame propagation of methane-air mixture in a closed tube is estimated through a direct numerical simulation of the three-dimensional unsteady Navier-Stokes equations coupled with chemical reaction. In order to deal with a combusting flow, an extended version of the MAC method, which can be applied to a compressible flow with strong density variation, is employed as a numerical method. The chemical reaction is assumed to be an irreversible single step reaction between methane and oxygen. The chemical species are CH 4, O 2, N 2, CO 2, and H 2O. In this simulation, we reproduce a formation of a tulip flame in a closed tube during the flame propagation. Furthermore we estimate not only a two-dimensional shape but also a three-dimensional structure of the flame and flame-induced vortices, which cannot be observed in the experiments. The agreement between the calculated results and the experimental data is satisfactory, and we compare the phenomenon near the side wall with the one in the corner of the tube.

  13. Fundamental mechanisms in premixed flame propagation via vortex-flame interactions: Numerical simulations

    NASA Technical Reports Server (NTRS)

    Mantel, Thierry

    1994-01-01

    The goal of the present study is to assess numerically the ability of single-step and two-step chemical models to describe the main features encountered during the interaction between a two-dimensional vortex pair and a premixed laminar flame. In the two-step mechanism, the reaction kinetics are represented by a first chain branching reaction A + X yields 2X and a second chain termination reaction X + X yields P. This paper presents the fundamental mechanisms occurring during vortex-flame interactions and the relative impact of the major parameters encountered in turbulent premixed flames and suspected of playing a role in quenching mechanism: (1) Influence of stretch is investigated by analyzing the contribution of curvature and tangential strain on the local structure of the flame. The effect of Lewis number on the flame response to a strained field is analyzed. (2) Radiative heat losses which are suspected to be partially or totally responsible for quenching are also investigated. (3) The effect of the diffusion of the radicals is studied using a two-step mechanism in which an intermediate species is present. The parameters of the two-step mechanism are entirely determined from physical arguments. (4) Precise quantitative comparisons between the DNS and the experimental results of Samaniego et al are performed. These comparisons concern the evolution of the minimum heat release rate found along the flame front during the interaction and the distribution of the heat release rate along the flame front.

  14. Catalysis of propane oxidation and premixed propane-air flames

    NASA Astrophysics Data System (ADS)

    Wiswall, James T.

    Improvements in deriving energy from hydrocarbon fuels will have a large impact on our efforts to transition to sustainable and renewable energy resources. The hypothesis for this work is that catalysis can extend the useful operating conditions for hydrocarbon oxidation and combustion, improve device efficiencies, and reduce pollutants. Catalysis of propane oxidation and premixed propane-air flames are examined experimentally, using a stagnation-flow reactor to identify the important physical and chemical mechanisms over a range of flow catalyst, and temperature conditions. The propane oxidation studies consider five catalyst materials: platinum, palladium, SnO2, 90% SnO2 -- 10% Pt (by mass), and quartz. The volume fractions of CO2, O2, C 3H8, CO, NO and the electric power required to control the catalyst temperature quantify the activity of each catalyst for the equivalence ratios of φ = 0.67, 1.00, and 1.50, and over the catalyst temperature range 23-800°C. Quartz is used as a baseline and confirmed to be non-reactive at all conditions. 100% SnO2 has minimal reactivity. Platinum, palladium, and 90% SnO2 -- 10% Pt show similar trends and have the highest catalytic activity at φ = 1.50. Palladium and 90% SnO 2 -- 10% Pt show an increasing catalyst-activation temperature (Tsa) for decreasing φ, and platinum shows an approximately constant catalyst-activation temperature for decreasing φ (Tsa = 310°C). Of these the 90% SnO2 -- 10% Pt catalyst shows the lowest Tsa, occurring for the φ = 1.5 mixture (Tsa = 250°C). The studies of premixed propane-air flames consider platinum and quartz stagnation surfaces for fuel-mixture velocities from 0.6-1.6 m/s. Five flame structures are observed: cool core envelope, cone, envelope, disk and ring flames. The lean-extinction limit, disk-to-ring flame transition φ, and the disk-flame to stagnation-plane distance are reported. Platinum inhibits the ring flame structure. The lean-extinction limit and disk-flame to stagnation

  15. Some effects of gravity on the behavior of premixed flames

    SciTech Connect

    Durvox, D.; Baillot, F.; Seouflaire, P.; Prudhomme, R. )

    1990-10-01

    This paper reports how, in ground-level tests on Bunsen-type premixed flames, a vertical fixed-frequency pumping effect can be observed at the tip of the flame, provided the latter is tall enough and the flow is laminar at the burner outlet. The effect vanishes completely under the microgravity conditions prevailing during parabolic flight tests, when natural convection no longer exists; in contrast, pumping frequency becomes higher as the acceleration of gravity increases. In a recent parabolic flight program, the frequency increase was measured while the aircraft was climbing at 1.8 g acceleration. Flight tests were supplemented by ground testing to derive the law of the frequency change as a function of pressure, equivalence ratio and flow velocity.

  16. Study on the premixed laminar flames of iso-octane

    NASA Astrophysics Data System (ADS)

    Yang, Bo; Hong, Yan-ji; Xu, Qing-yao; Liu, Yi; Cheng, Qi-sheng; Ding, Xiao-yu

    2015-04-01

    Propagation characteristics of premixed laminar iso-octane flames at atmosphere and equivalence ratios from 0.8 to 1.4 are studied in a constant combustion bomb using a schlieren technique, the laminar burning velocity at different initial pressure, temperature, equivalence ratio are calculated through CHEMKIN program. The experimental and calculation results show that the laminar burning velocity of iso-octane rise with the decreasing of initial pressure and rise with the rising of initial temperature . Only changing the initial temperature or pressure ,the maximum laminar burning velocity of iso-octane were both obtained at equivalence ratio 1.1. Flame stability become weak ,when increased the equivalence ratio. The problem of the chemistry reaction mechanism to predict the laminar burning velocity were analysed.

  17. Lewis number effects on turbulent premixed flame structure

    SciTech Connect

    Goix, P.J. , 230 - Mont-Saint-Aignan . URA CORIA); Shepherd, I.G. )

    1992-09-01

    The influence of the Lewis number on turbulent flame front geometry is investigated in a premixed turbulent stagnation point flame. A laser tomography technique is used to obtain the flame shape, a fractal analysis of the multiscale flame edges is performed and the distribution of local flame front curvature is determined. Lean H[sub 2]/Air and C[sub 3]H[sub 8]/Air mixtures with similar burning rates were investigated with Lewis numbers of 0.33 and 1.85 respectively. At the conditions studied the laminar H[sub 2]/Air mixture is unstable and a cellular structure is observed. Turbulence in the reactant is generated by a perforated plate and the turbulent length scale (3mm) and intensity (7%) at the nozzle exit are fixed. The equivalence ratio is set so that the burning velocity is the same for all the cases. Results show clearly that the turbulent flame surface area is dependent on the Lewis number. For a Lewis number less than unity surface area production is observed. The shape of the flame front curvature distribution is not found to be very sensitive to the Lewis number. For the H[sub 2]/Air mixture the distribution is skewed toward the positive values indicating the presence of cusps while for the C[sub 3]H[sub 8]/Air mixture the distribution is more symmetrical. In both cases the average curvature is found to be zero, and if the local burning speed varies linearly with curvature, the local positive and negative burning velocity variations due to curvature will balance.

  18. Lewis number effects on turbulent premixed flame structure

    SciTech Connect

    Goix, P.J.; Shepherd, I.G.

    1992-09-01

    The influence of the Lewis number on turbulent flame front geometry is investigated in a premixed turbulent stagnation point flame. A laser tomography technique is used to obtain the flame shape, a fractal analysis of the multiscale flame edges is performed and the distribution of local flame front curvature is determined. Lean H{sub 2}/Air and C{sub 3}H{sub 8}/Air mixtures with similar burning rates were investigated with Lewis numbers of 0.33 and 1.85 respectively. At the conditions studied the laminar H{sub 2}/Air mixture is unstable and a cellular structure is observed. Turbulence in the reactant is generated by a perforated plate and the turbulent length scale (3mm) and intensity (7%) at the nozzle exit are fixed. The equivalence ratio is set so that the burning velocity is the same for all the cases. Results show clearly that the turbulent flame surface area is dependent on the Lewis number. For a Lewis number less than unity surface area production is observed. The shape of the flame front curvature distribution is not found to be very sensitive to the Lewis number. For the H{sub 2}/Air mixture the distribution is skewed toward the positive values indicating the presence of cusps while for the C{sub 3}H{sub 8}/Air mixture the distribution is more symmetrical. In both cases the average curvature is found to be zero, and if the local burning speed varies linearly with curvature, the local positive and negative burning velocity variations due to curvature will balance.

  19. Time-dependent Computational Studies of Premixed Flames in Microgravity

    NASA Technical Reports Server (NTRS)

    Kailasanath, K.; Patnaik, Gopal; Oran, Elaine S.

    1993-01-01

    This report describes the research performed at the Center for Reactive Flow and Dynamical Systems in the Laboratory for Computational Physics and Fluid Dynamics, at the Naval Research Laboratory, in support of NASA Microgravity Science and Applications Program. The primary focus of this research is on investigating fundamental questions concerning the propagation and extinction of premixed flames in earth gravity and in microgravity environments. Our approach is to use detailed time-dependent, multispecies, numerical models as tools to simulate flames in different gravity environments. The models include a detailed chemical kinetics mechanism consisting of elementary reactions among the eight reactive species involved in hydrogen combustion, coupled to algorithms for convection, thermal conduction, viscosity, molecular and thermal diffusion, and external forces. The external force, gravity, can be put in any direction relative to flame propagation and can have a range of values. Recently more advanced wall boundary conditions such as isothermal and no-slip have been added to the model. This enables the simulation of flames propagating in more practical systems than before. We have used the numerical simulations to investigate the effects of heat losses and buoyancy forces on the structure and stability of flames, to help resolve fundamental questions on the existence of flammability limits when there are no external losses or buoyancy forces in the system, to understand the interaction between the various processes leading to flame instabilities and extinguishment, and to study the dynamics of cell formation and splitting. Our studies have been able to bring out the differences between upward- and downward-propagating flames and predict the zero-gravity behavior of these flames. The simulations have also highlighted the dominant role of wall heat losses in the case of downward-propagating flames. The simulations have been able to qualitatively predict the

  20. Experimental study on the flame behaviors of premixed methane/air mixture in horizontal rectangular ducts

    NASA Astrophysics Data System (ADS)

    Chen, Dongliang; Sun, Jinhua; Chen, Sining; Liu, Yi; Chu, Guanquan

    2007-01-01

    In order to explore the flame propagation characteristics and tulip flame formation mechanism of premixed methane/air mixture in horizontal rectangular ducts, the techniques of Schlieren and high-speed video camera are used to study the flame behaviors of the premixed gases in a closed duct and opened one respectively, and the propagation characteristics in both cases and the formation mechanism of the tulip flame are analyzed. The results show that, the propagation flame in a closed duct is prior to form a tulip flame structure than that in an opened duct, and the tulip flame structure formation in a closed duct is related to the flame propagation velocity decrease. The sharp decrease of the flame propagation velocity is one of the reasons to the tulip flame formation, and the decrease of the flame propagation velocity is due to the decrease of the burned product flow velocity mainly.

  1. Multiple mapping conditioning for flames with partial premixing

    SciTech Connect

    Kronenburg, A.; Cleary, M.J.

    2008-10-15

    Fully closed multiple mapping conditioning (MMC) is used to model partially premixed flames in homogeneous, isotropic decaying turbulence where the partial premixing is caused by local extinction and reignition phenomena. Two reference variables that represent mixing and reaction progress, such as mixture fraction and sensible enthalpy, are used to emulate turbulent scalar fluctuations. Local extinction is achieved by a priori coupling between scalar dissipation and temperature fluctuations via a correlation function that is based on the conditionally averaged sensible enthalpy at stoichiometric composition. The proposed model provides closures for the joint PDF of mixture fraction and sensible enthalpy, for the conditional variance equation of a reactive scalar, and for the doubly conditioned dissipation terms. Model results are compared with DNS in three flame cases with varying levels of local extinction, up to global extinction. The joint PDF predicted by MMC is in fair agreement with DNS. It constitutes, however, a clear improvement over conventional models using preassumed distribution functions for the PDFs. The doubly conditioned dissipation terms are modeled well and the results for all major chemical species are in good agreement with DNS. Predictions for intermediate species are also satisfactory. (author)

  2. Effect of turbulence characteristics on local flame structure of H2 air premixed flames

    NASA Astrophysics Data System (ADS)

    Nada, Y.; Tanahashi, M.; Miyauchi, T.

    2004-04-01

    Direct numerical simulations (DNS) of turbulent premixed flames are conducted to investigate effects of turbulence characteristics on the local flame structure. A detailed kinetic mechanism including 12 reactive species and 27 elementary reactions is used to represent the H2-air reaction in turbulence. Numerical conditions of DNS can be classified into a wrinkled-flamelets regime, a corrugated-flamelets regime and thin reaction zones near the boundary of Karlovitz number Ka=1.0 of the turbulent-combustion diagram. For all cases, the distribution of heat-release rate shows a three-dimensionally connected sheet-like feature, even though the heat-release rate highly fluctuates along the flamefront. The heat-release rate tends to increase at the flamefronts that are convex towards the burnt side. For the turbulent premixed flames in the corrugated-flamelets regime, the handgrip structure is produced by the intrusion of the coherent fine-scale eddy into the flame and the heat-release rate in this structure increases up to 1.2 times of that of a laminar flame. In the wrinkled-flamelets regime, the spire-like structure of the flamefront is created due to the coherent fine-scale eddies in turbulence. By identifying flame elements in turbulence, their statistical characteristics are also discussed. This article was chosen from Selected Proceedings of the Third International Symposium on Turbulence and Shear Flow Phenomena (Sendai, Japan, 24-27 June 2003) ed N Kasagi et al.

  3. Rayleigh-Taylor Instability in non-premixed reacting flames.

    NASA Astrophysics Data System (ADS)

    Attal, Nitesh; Ramaprabhu, Praveen

    2015-11-01

    The Rayleigh-Taylor instability (RTI) occurs at a perturbed interface between fluids of different densities when a light fluid pushes a heavier fluid. The mixing driven by RTI affects several physical phenomena, such as Inertial Confinement Fusion, Supernovae detonation, centrifugal combustors and liquid rocket engines. The RTI in such flows is often coupled with chemical/nuclear reactions that may form complex density stratifications in the form of flames or ablative layers. We investigate such a non-premixed fuel-air interface subject to a constant acceleration and developing under the influence of chemical reactions using high-resolution, Navier-Stokes simulations. The H2 fuel is diluted with N2 to vary the density difference across the interface in thermal equilibrium (at 1000K). The intervening layer between fuel and air is subject to exothermic combustion reactions to form a flame. Following combustion, initially unstable fuel-air interfaces at an Atwood number (At) <0.5, transform into stable (fuel-flame) and unstable (flame-air) interfaces. We report on interfaces (At = 0.2 and 0.6) with single wavelength, sinusoidal perturbations and a broadband spectrum of multimode perturbations.

  4. Partially-Premixed Flames in Internal Combustion Engines

    SciTech Connect

    Robert W. Pitz; Michael C. Drake; Todd D. Fansler; Volker Sick

    2003-11-05

    This was a joint university-industry research program funded by the Partnerships for the Academic-Industrial Research Program (PAIR). The research examined partially premixed flames in laboratory and internal combustion engine environments at Vanderbilt University, University of Michigan, and General Motors Research and Development. At Vanderbilt University, stretched and curved ''tubular'' premixed flames were measured in a unique optically accessible burner with laser-induced spontaneous Raman scattering. Comparisons of optically measured temperature and species concentration profiles to detailed transport, complex chemistry simulations showed good correspondence at low-stretch conditions in the tubular flame. However, there were significant discrepancies at high-stretch conditions near flame extinction. The tubular flame predictions were found to be very sensitive to the specific hydrogen-air chemical kinetic mechanism and four different mechanisms were compared. In addition, the thermo-diffusive properties of the deficient reactant, H2, strongly affected the tubular flame structure. The poor prediction near extinction is most likely due to deficiencies in the chemical kinetic mechanisms near extinction. At the University of Michigan, an optical direct-injected engine was built up for laser-induced fluorescence imaging experiments on mixing and combustion under stratified charge combustion conditions with the assistance of General Motors. Laser attenuation effects were characterized both experimentally and numerically to improve laser imaging during the initial phase of the gasoline-air mixture development. Toluene was added to the isooctane fuel to image the fuel-air equivalence ratio in an optically accessible direct-injected gasoline engine. Temperature effects on the toluene imaging of fuel-air equivalence ratio were characterized. For the first time, oxygen imaging was accomplished in an internal combustion engine by combination of two fluorescence trackers

  5. Measurements and modeling of nitric oxide formation in counterflow, premixed, methane/oxygen/nitrogen flames

    NASA Astrophysics Data System (ADS)

    Thomsen, Duane Douglas

    1999-10-01

    Laser-induced fluorescence (LIF) measurements of NO concentration in a variety of CH4/O2/N2 flames are used to evaluate the chemical kinetics of NO formation. The analysis begins with previous measurements in flat, laminar, premixed CH4/O2/N 2 flames stabilized on a water-cooled McKenna burner at pressures ranging from 1 to 14.6 atm, equivalence ratios from 0.5 to 1.6, and volumetric nitrogen/oxygen dilution ratios of 2.2, 3.1 and 3.76. These measured results are compared to predictions to determine the capabilities and limitations of the comprehensive kinetic mechanism developed by the Gas Research Institute (GRI), version 2.11. The model is shown to predict well the qualitative trends of NO formation in lean-premixed flames, while quantitatively underpredicting NO concentration by 30-50%. For rich flames, the model is unable to even qualitatively match the experimental results. These flames were found to be limited by low temperatures and an inability to separate the flame from the burner surface. In response to these limitations, a counterflow burner was designed for use in opposed premixed flame studies. A new LIF calibration technique was developed and applied to obtain quantitative measurements of NO concentration in laminar, counterflow premixed, CH 4/O2/N2 flames at pressures ranging from 1 to 5.1 atm, equivalence ratios of 0.6 to 1.5, and an N2/O2 dilution ratio of 3.76. The counterflow premixed flame measurements are combined with measurements in burner-stabilized premixed flames and counterflow diffusion flames to build a comprehensive database for analysis of the GRI kinetic mechanism. Pathways, quantitative reaction path and sensitivity analyses are applied to the GRI mechanism for these flame conditions. The prompt NO mechanism is found to severely underpredict the amount of NO formed in rich premixed and nitrogen-diluted diffusion flames. This underprediction is traced to uncertainties in the CH kinetics as well as in the nitrogen oxidation chemistry

  6. The Behavior of Methane-Air Partially Premixed Flames Under Normal- and Zero-G Conditions

    NASA Technical Reports Server (NTRS)

    Puri, Ishwar K.; Aggarwal, Suresh K.; Choi, Chun Wai; Hegde, Uday

    2001-01-01

    Partially premixed flames (PPFs) represent a class of hybrid flames containing multiple reaction zones. These flames are established when less than stoichiometric quantity of oxidizer is molecularly mixed with the fuel stream before entering the reaction zone where additional oxidizer is available for complete combustion. This mode of combustion can be used to exploit the advantages of both nonpremixed and premixed flames regarding operational safety, lower pollutant emissions and flame stabilization. A double flame containing a fuel-rich premixed reaction zone, which is anchored by a nonpremixed reaction zone, is one example of a partially premixed flame. A triple flame is also a PPF that contains three reaction zones, namely, a fuel-rich premixed zone, a fuel-lean premixed zone, and a nonpremixed reaction zone. Herein we focus on two aspects of our investigation, one involving the development of optical diagnostics that can be used on a microgravity rig, which has been recently fabricated, and the other on the numerically predicted differences between normal- and zero-gravity PPFs. Both the measurements and simulations examine the detailed structure of methane-air PPFs stabilized on a Wolfhard-Parker slot burner.

  7. Numerical computations and optical diagnostics of unsteady partially premixed methane/air flames

    SciTech Connect

    Nogenmyr, K.J.; Bai, X.S.; Kiefer, J.; Li, Z.S.; Alden, M.

    2010-05-15

    The structures and dynamics of unsteady laminar partially premixed methane/air Bunsen flames are studied by means of numerical simulations, OH and CH PLIF imaging, and high speed chemiluminescence imaging employing a high framing speed intensified charge coupled device camera. The Bunsen burner has a diameter of 22 mm. Rich methane/air mixtures with an equivalence ratio of 1.5 are injected from the burner into atmosphere at different flow speeds ranging from 0.77 to 1.7 m/s, with Reynolds numbers based on the nozzle flow ranging from 1100 to 2500. The numerical simulations are based on a two-scalar flamelet manifold tabulation approach. Detailed chemistry is used to generate the flamelet manifold tabulation which relates the species concentrations, reaction rates, temperature and density to a distance function G and mixture fraction Z. Two distinct reaction zones are identified using CH and OH PLIF imaging and numerical simulations; one inner reaction zone corresponds to premixed flames on the rich side of the mixture and one outer reaction zone corresponds to mixing controlled diffusion flames on the lean side of the mixture. Under normal gravity conditions both the inner premixed flames and the outer diffusion flames are unsteady. The outer diffusion flames oscillate with a flickering frequency of about 15 Hz, which slightly increases with the burner exit velocity. The inner premixed flames are more random with much more small-scale wrinkling structures. Under zero gravity conditions the outer diffusion flames are stable whereas the inner premixed flames are unstable and highly wrinkled. It appears that the outer diffusion flames are governed by the Rayleigh-Taylor instability whereas the inner premixed flames are dictated by Landau-Darrieus instability. The two-scalar flamelet approach is shown to capture the basic structures and dynamics of the investigated unsteady partially premixed flames. (author)

  8. Effect of dilatation on scalar dissipation in turbulent premixed flames

    SciTech Connect

    Swaminathan, N.; Bray, K.N.C.

    2005-12-01

    The scalar dissipation rate signifies the local mixing rate and thus plays a vital role in the modeling of reaction rate in turbulent flames. The local mixing rate is influenced by the turbulence, the chemical, and the molecular diffusion processes which are strongly coupled in turbulent premixed flames. Thus, a model for the mean scalar dissipation rate, and hence the mean reaction rate, should include the contributions of these processes. Earlier models for the scalar dissipation rate include only a turbulence time scale. In this study, we derive exact transport equations for the instantaneous and the mean scalar dissipation rates. Using these equations, a simple algebraic model for the mean scalar dissipation rate is obtained. This model includes a chemical as well as a turbulence time scale and its prediction compares well with direct numerical simulation results. Reynolds-averaged Navier-Stokes calculations of a test flame using the model obtained here show that the contribution of dilatation to local turbulent mixing rate is important to predict the propagation phenomenon.

  9. Simultaneous velocity and scalar measurements in premixed recirculating flames

    NASA Astrophysics Data System (ADS)

    Ferrão, P.; Heitor, M. V.

    The use of a laser-Doppler velocimeter has been extended to the analysis of turbulent heat transfer in a strongly sheared disc-stabilised propane-air flame through its combination with either laser Rayleigh scattering or digitally-compensated fine-wire thermocouples. The laser velocimeter was based on a conventional forward scattering system from the green light of a 5W Argon-Ion laser, while the Rayleigh signals used the blue line of the same laser. The procedure for the numeric compensation of the thermocouple signals included analysis of the effect of velocity and temperature on the time constant of the thermocouple and was optimised to allow combined velocity-temperature samples acquired by a purpose-built digital interference with a frequency up to 2000 Hz, without deterioration of the thermocouple by particle accretion. The maximum effective data rate for the combined Rayleigh/LDV system is shown to be around 130 Hz, which corresponds to a data rate of valid Doppler signals around 400 Hz and statistics based on more than 15000 measurements is made possible. The results obtained with the two systems agree qualitatively, although the use of thermocouples attenuates the measured velocity-temperature correlations. The results are used to assess the extent to which turbulent mixing in flames is altered by the accompanying heat release and quantify the processes of non-gradient diffusion in a strongly recirculating premixed flame.

  10. Soot Formation in Purely-Curved Premixed Flames and Laminar Flame Speeds of Soot-Forming Flames

    NASA Technical Reports Server (NTRS)

    Buchanan, Thomas; Wang, Hai

    2005-01-01

    The research addressed here is a collaborative project between University of Delaware and Case Western Reserve University. There are two basic and related scientific objectives. First, we wish to demonstrate the suitability of spherical/cylindrical, laminar, premixed flames in the fundamental study of the chemical and physical processes of soot formation. Our reasoning is that the flame standoff distance in spherical/cylindrical flames under microgravity can be substantially larger than that in a flat burner-stabilized flame. Therefore the spherical/cylindrical flame is expected to give better spatial resolution to probe the soot inception and growth chemistry than flat flames. Second, we wish to examine the feasibility of determining the laminar flame speed of soot forming flames. Our basic assumption is that under the adiabatic condition (in the absence of conductive heat loss), the amount and dynamics of soot formed in the flame is unique for a given fuel/air mixture. The laminar flame speed can be rigorously defined as long as the radiative heat loss can be determined. This laminar flame speed characterizes the flame soot formation and dynamics in addition to the heat release rate. The research involves two integral parts: experiments of spherical and cylindrical sooting flames in microgravity (CWRU), and the computational counterpart (UD) that aims to simulate sooting laminar flames, and the sooting limits of near adiabatic flames. The computations work is described in this report, followed by a summary of the accomplishments achieved to date. Details of the microgra+ experiments will be discussed in a separate, final report prepared by the co-PI, Professor C-J. Sung of CWRU. Here only a brief discussion of these experiments will be given.

  11. PREMIXED FLAME PROPAGATION AND MORPHOLOGY IN A CONSTANT VOLUME COMBUSTION CHAMBER

    SciTech Connect

    Hariharan, A; Wichman, IS

    2014-06-04

    This work presents an experimental and numerical investigation of premixed flame propagation in a constant volume rectangular channel with an aspect ratio of six (6) that serves as a combustion chamber. Ignition is followed by an accelerating cusped finger-shaped flame-front. A deceleration of the flame is followed by the formation of a "tulip"-shaped flame-front. Eventually, the flame is extinguished when it collides with the cold wall on the opposite channel end. Numerical computations are performed to understand the influence of pressure waves, instabilities, and flow field effects causing changes to the flame structure and morphology. The transient 2D numerical simulation results are compared with transient 3D experimental results. Issues discussed are the appearance of oscillatory motions along the flame front and the influences of gravity on flame structure. An explanation is provided for the formation of the "tulip" shape of the premixed flame front.

  12. Turbulent premixed combustion in V-shaped flames: Characteristics of flame front

    NASA Astrophysics Data System (ADS)

    Kheirkhah, S.; Gülder, Ö. L.

    2013-05-01

    Flame front characteristics of turbulent premixed V-shaped flames were investigated experimentally using the Mie scattering and the particle image velocimetry techniques. The experiments were performed at mean streamwise exit velocities of 4.0, 6.2, and 8.6 m/s, along with fuel-air equivalence ratios of 0.7, 0.8, and 0.9. Effects of vertical distance from the flame-holder, mean streamwise exit velocity, and fuel-air equivalence ratio on statistics of the distance between the flame front and the vertical axis, flame brush thickness, flame front curvature, and angle between tangent to the flame front and the horizontal axis were studied. The results show that increasing the vertical distance from the flame-holder and the fuel-air equivalence ratio increase the mean and root-mean-square (RMS) of the distance between the flame front and the vertical axis; however, increasing the mean streamwise exit velocity decreases these statistics. Spectral analysis of the fluctuations of the flame front position depicts that the normalized and averaged power-spectrum-densities collapse and show a power-law relation with the normalized wave number. The flame brush thickness is linearly correlated with RMS of the distance between the flame front and the vertical axis. Analysis of the curvature of the flame front data shows that the mean curvature is independent of the experimental conditions tested and equals to zero. Values of the inverse of the RMS of flame front curvature are similar to those of the integral length scale, suggesting that the large eddies in the flow make a significant contribution in wrinkling of the flame front. Spectral analyses of the flame front curvature as well as the angle between tangent to the flame front and the horizontal axis show that the power-spectrum-densities feature a peak. Value of the inverse of the wave number pertaining to the peak is larger than that of the integral length scale.

  13. RANS/PDF and LES/FDF for prediction of turbulent premixed flames

    NASA Astrophysics Data System (ADS)

    Yilmaz, Server Levent

    Probability density function (PDF) and filtered density function (FDF) methodologies are developed and implemented, respectively, for Reynolds-averaged Navier-Stokes (RANS) and large eddy simulation (LES) of turbulent premixed flames. RANS predictions are made of a lean premixed bluff-body flame via the joint velocity-scalar-frequency PDF model. LES of a premixed Bunsen-burner flame is conducted via the scalar FDF methodology. Both simulations employ finite rate kinetics via a reduced methane chemistry mechanism to account for combustion. Prediction results are compared with experimental data, and are shown to capture some of the intricate physics of turbulent premixed combustion. Keywords. large eddy simulation, filtered density function, Reynolds-averaged Navier-Stokes, probability density function, turbulent reacting flows, lean premixed combustion.

  14. The dynamics of turbulent premixed flames: Mechanisms and models for turbulence-flame interaction

    NASA Astrophysics Data System (ADS)

    Steinberg, Adam M.

    The use of turbulent premixed combustion in engines has been garnering renewed interest due to its potential to reduce NOx emissions. However there are many aspects of turbulence-flame interaction that must be better understood before such flames can be accurately modeled. The focus of this dissertation is to develop an improved understanding for the manner in which turbulence interacts with a premixed flame in the 'thin flamelet regime'. To do so, two new diagnostics were developed and employed in a turbulent slot Bunsen flame. These diagnostics, Cinema-Stereoscopic Particle Image Velocimetry and Orthogonal-Plane Cinema-Stereoscopic Particle Image Velocimetry, provided temporally resolved velocity and flame surface measurements in two- and three-dimensions with rates of up to 3 kHz and spatial resolutions as low as 280 mum. Using these measurements, the mechanisms with which turbulence generates flame surface area were studied. It was found that the previous concept that flame stretch is characterized by counter-rotating vortex pairs does not accurately describe real turbulence-flame interactions. Analysis of the experimental data showed that the straining of the flame surface is determined by coherent structures of fluid dynamic strain rate, while the wrinkling is caused by vortical structures. Furthermore, it was shown that the canonical vortex pair configuration is not an accurate reflection of the real interaction geometry. Hence, models developed based on this geometry are unlikely to be accurate. Previous models for the strain rate, curvature stretch rate, and turbulent burning velocity were evaluated. It was found that the previous models did not accurately predict the measured data for a variety of reasons: the assumed interaction geometries did not encompass enough possibilities to describe the possible effects of real turbulence, the turbulence was not properly characterized, and the transport of flame surface area was not always considered. New models

  15. Intermittent features of inertial particle distributions in turbulent premixed flames

    NASA Astrophysics Data System (ADS)

    Battista, F.; Picano, F.; Troiani, G.; Casciola, C. M.

    2011-12-01

    Clustering is widely observed in many turbulent flows, where it results from the inability of finite inertia particles to comply with the different time scales, which characterize a turbulent field. Depending on their inertia, particles are found to be instantaneously organized in clusters, whose size depends on the Kolmogorov-Stokes number and which presumably form as a consequence of particle ejection from persistent vortical structures. In reacting flows, the abrupt acceleration of the fluid across the thin flame front due to combustion adds new and unexpected features. The particles follow such acceleration with a certain time lag which, coupled with the flame front fluctuations, gives rise to an entirely different mechanism of cluster formation. As suggested in previous studies, a possible indicator of this preferential localization is the so-called clustering index, quantifying the departure of the actual particle arrangement from the Poissonian distribution. Most of the clustering is found in the flame brush region, where it cannot be explained by the standard arguments used in cold flows. Actually, the effect is significant also for very light particles, where the simple model we propose, based on the Bray-Moss-Libby formalism, is able to account for most of the deviation from the Poissonian. When the particle inertia increases, the effect becomes larger and it is found to persist well within the region of the burned gases. The observed clustering is confirmed by a more precise analysis in terms of a generalization of the radial distribution function to inhomogeneous, anisotropic flows. The results taken from a direct numerical simulation with single step kinetics favorably compare with experiments on a premixed Bunsen turbulent flame. The present findings are expected to be of some relevance for the plenty of applications dealing with particles in presence of combustion, e.g., liquid droplet swarms for combustion temperature control, soot dynamics, or

  16. An Investigation of a Hybrid Mixing Model for PDF Simulations of Turbulent Premixed Flames

    NASA Astrophysics Data System (ADS)

    Zhou, Hua; Li, Shan; Wang, Hu; Ren, Zhuyin

    2015-11-01

    Predictive simulations of turbulent premixed flames over a wide range of Damköhler numbers in the framework of Probability Density Function (PDF) method still remain challenging due to the deficiency in current micro-mixing models. In this work, a hybrid micro-mixing model, valid in both the flamelet regime and broken reaction zone regime, is proposed. A priori testing of this model is first performed by examining the conditional scalar dissipation rate and conditional scalar diffusion in a 3-D direct numerical simulation dataset of a temporally evolving turbulent slot jet flame of lean premixed H2-air in the thin reaction zone regime. Then, this new model is applied to PDF simulations of the Piloted Premixed Jet Burner (PPJB) flames, which are a set of highly shear turbulent premixed flames and feature strong turbulence-chemistry interaction at high Reynolds and Karlovitz numbers. Supported by NSFC 51476087 and NSFC 91441202.

  17. The detailed flame structure of highly stretched turbulent premixed methane-air flames

    SciTech Connect

    Chen, Y.C.; Peters, N.; Schneemann, G.A.; Wruck, N.; Renz, U.; Mansour, M.S.

    1996-11-01

    The premixed stoichiometric turbulent methane flames are investigated on a piloted Bunsen burner with mean nozzle exit velocities of 65, 50, and 30 m/s. Advanced laser diagnostics of the flow field using two-component and two-point laser Doppler anemometer, as well as of the scalar fields with 2-D Rayleigh thermometry and line Raman/Rayleigh laser-induced predissociation fluorescence techniques, are applied to obtain both the instantaneous and mean flame structure in terms of velocity, temperature, and major species concentrations, as well as turbulent kinetic energy and length scales. The three flames cover the entire range of the distributed-reaction-zones regime from the borderline to the well-stirred reactor regime to the flamelet regime. Measurements were from X/D = 2.5 above the nozzle exit plane to X/D = 12.5 downstream. Thus, a complete database is established for comparison with the numerical predictions. Within the mixing layer between the unburnt gas and the pilot flame, the instantaneous temperatures are much lower than the adiabatic flame temperature due to the short residence time and heat loss to the burner. With increasing residence time the mean flame temperature increases in the axial direction. The radial mixing of the turbulence generated with the shear layers between the nozzle jet stream and surrounding pilot stream is suppressed, such that the turbulence kinetic energy remains nearly constant on the centerline. From the two-dimensional temperature fields instantaneous iso-temperature contours are plotted showing broad regions where burnt and unburnt gas are partially mixed. These regions are interpreted in terms of the quench scale {ell}{sub q} = ({epsilon}{tau}{sub c}{sup 3}){sup 1/2}. The measured values of the flame brush thickness are proportional to the quench scale for the two high-velocity flames, whereas the low-velocity flame exhibits essential flamelet behavior.

  18. Turbulence-flame interactions in DNS of a laboratory high Karlovitz premixed turbulent jet flame

    NASA Astrophysics Data System (ADS)

    Wang, Haiou; Hawkes, Evatt R.; Chen, Jacqueline H.

    2016-09-01

    In the present work, direct numerical simulation (DNS) of a laboratory premixed turbulent jet flame was performed to study turbulence-flame interactions. The turbulent flame features moderate Reynolds number and high Karlovitz number (Ka). The orientations of the flame normal vector n, the vorticity vector ω and the principal strain rate eigenvectors ei are examined. The in-plane and out-of-plane angles are introduced to quantify the vector orientations, which also measure the flame geometry and the vortical structures. A general observation is that the distributions of these angles are more isotropic downstream as the flame and the flow become more developed. The out-of-plane angle of the flame normal vector, β, is a key parameter in developing the correction of 2D measurements to estimate the corresponding 3D quantities. The DNS results show that the correction factor is unity at the inlet and approaches its theoretical value of an isotropic distribution downstream. The alignment characteristics of n, ω and ei, which reflect the interactions of turbulence and flame, are also studied. Similar to a passive scalar gradient in non-reacting flows, the flame normal has a tendency to align with the most compressive strain rate, e3, in the flame, indicating that turbulence contributes to the production of scalar gradient. The vorticity dynamics are examined via the vortex stretching term, which was found to be the predominant source of vorticity generation balanced by dissipation, in the enstrophy transport equation. It is found that although the vorticity preferentially aligns with the intermediate strain rate, e2, the contribution of the most extensive strain rate, e1, to vortex stretching is comparable with that of the intermediate strain rate, e2. This is because the eigenvalue of the most extensive strain rate, λ1, is always large and positive. It is confirmed that the vorticity vector is preferentially positioned along the flame tangential plane, contributing

  19. Tabulated Combustion Model Development For Non-Premixed Flames

    NASA Astrophysics Data System (ADS)

    Kundu, Prithwish

    Turbulent non-premixed flames play a very important role in the field of engineering ranging from power generation to propulsion. The coupling of fluid mechanics and complicated combustion chemistry of fuels pose a challenge for the numerical modeling of these type of problems. Combustion modeling in Computational Fluid Dynamics (CFD) is one of the most important tools used for predictive modeling of complex systems and to understand the basic fundamentals of combustion. Traditional combustion models solve a transport equation of each species with a source term. In order to resolve the complex chemistry accurately it is important to include a large number of species. However, the computational cost is generally proportional to the cube of number of species. The presence of a large number of species in a flame makes the use of CFD computationally expensive and beyond reach for some applications or inaccurate when solved with simplified chemistry. For highly turbulent flows, it also becomes important to incorporate the effects of turbulence chemistry interaction (TCI). The aim of this work is to develop high fidelity combustion models based on the flamelet concept and to significantly advance the existing capabilities. A thorough investigation of existing models (Finite-rate chemistry and Representative Interactive Flamelet (RIF)) and comparative study of combustion models was done initially on a constant volume combustion chamber with diesel fuel injection. The CFD modeling was validated with experimental results and was also successfully applied to a single cylinder diesel engine. The effect of number of flamelets on the RIF model and flamelet initialization strategies were studied. The RIF model with multiple flamelets is computationally expensive and a model was proposed on the frame work of RIF. The new model was based on tabulated chemistry and incorporated TCI effects. A multidimensional tabulated chemistry database generation code was developed based on the 1

  20. Effects of heat conduction and radical quenching on premixed stagnation flame stabilised by a wall

    NASA Astrophysics Data System (ADS)

    Zhang, Huangwei; Chen, Zheng

    2013-08-01

    The premixed stagnation flame stabilised by a wall is analysed theoretically considering thermally sensitive intermediate kinetics. We consider the limit case of infinitely large activation energy of the chain-branching reaction, in which the radical is produced infinitely fast once the cross-over temperature is reached. Under the assumptions of potential flow field and constant density, the correlation for flame position and stretch rate of the premixed stagnation flame is derived. Based on this correlation, the effects of heat conduction and radical quenching on the wall surface are examined. The wall temperature is shown to have great impact on flame bifurcation and extinction, especially when the flame is close to the wall. Different flame structures are observed for near-wall normal flame, weak flame, and critically quenched flame. The fuel and radical Lewis numbers are found to have opposite effects on the extinction stretch rate. Moreover, it is also demonstrated that only when the flame is close to the wall does the radical quenching strongly influence the flame bifurcation and extinction. The extinction stretch rate is shown to decrease with the amount of radical quenching for different fuel and radical Lewis numbers. Besides, the coupling between the wall heat conduction and radical quenching is found to greatly influence the bifurcation and extinction of the premixed stagnation flame.

  1. Liftoff characteristics of partially premixed flames under normal and microgravity conditions

    SciTech Connect

    Lock, Andrew J.; Briones, Alejandro M.; Aggarwal, Suresh K.; Qin, Xiao; Puri, Ishwar K.; Hegde, Uday

    2005-11-01

    An experimental and computational investigation on the liftoff characteristics of laminar partially premixed flames (PPFs) under normal (1-g) and microgravity ({mu}-g) conditions is presented. Lifted methane-air PPFs were established in axisymmetric coflowing jets using nitrogen dilution and various levels of partial premixing. The {mu}-g experiments were conducted in the 2.2-s drop tower at the NASA Glenn Research Center. A time-accurate, implicit algorithm that uses a detailed description of the chemistry and includes radiation effects is used for the simulations. The predictions are validated through a comparison of the flame reaction zone topologies, liftoff heights, lengths, and oscillation frequencies. The effects of equivalence ratio, gravity, jet velocity, and radiation on flame topology, liftoff height, flame length, base structure, and oscillation frequency are characterized. Both the simulations and measurements indicate that under identical conditions, a lifted {mu}-g PPF is stabilized closer to the burner compared with the 1-g flame, and that the liftoff heights of both 1-g and {mu}-g flames decrease with increasing equivalence ratio and approach their respective nonpremixed flame limits. The liftoff height also increases as the jet velocity is increased. In addition, the flame base structure transitions from a triple- to a double-flame structure as the flame liftoff height decreases. A modified flame index is developed to distinguish between the rich premixed, lean premixed, and nonpremixed reaction zones near the flame base. The 1-g lifted flames exhibit well-organized oscillations due to buoyancy-induced instability, while the corresponding {mu}-g flames exhibit steady-state behavior. The effect of thermal radiation is to slightly decrease the liftoff heights of both 1-g and {mu}-g flames under coflow conditions.

  2. Extinction and near-extinction instability of non-premixed tubular flames

    SciTech Connect

    Hu, Shengteng; Pitz, Robert W.; Yu, Wang

    2009-01-15

    Tubular non-premixed flames are formed by an opposed tubular burner, a new tool to study the effects of curvature on extinction and flame instability of non-premixed flames. Extinction of the opposed tubular flames generated by burning diluted H{sub 2}, CH{sub 4} or C{sub 3}H{sub 8} with air is investigated for both concave and convex curvature. To examine the effects of curvature on extinction, the critical fuel dilution ratios at extinction are measured at various stretch rates, initial mixture strengths and flame curvature for fuels diluted in N{sub 2}, He, Ar or CO{sub 2}. In addition, the onset conditions of the cellular instability are mapped as a function of stretch rates, initial mixture strengths, and flame curvature. For fuel mixtures with Lewis numbers much less than unity, such as H{sub 2}/N{sub 2}, concave flame curvature towards the fuel suppresses cellular instabilities. (author)

  3. The influence of Lewis number and nonhomogeneous mixture on premixed turbulent flame structure

    NASA Technical Reports Server (NTRS)

    Haworth, D. C.; Poinsot, T. J.

    1990-01-01

    The structure of a premixed flame front in two-dimensional turbulence is investigated using full numerical simulation including heat release, variable fluid properties, and one-step Arrhenius chemistry. Non-unity Lewis number (Le) effects are described by comparing the local instantaneous turbulent flame structure to the steady one dimensional laminar flame structure for the same thermochemical parameters. Flame surface area, mean reactant consumption rate per unit area of flame, turbulent flame speed, and statistical descriptions of the flame geometry are also reported. Principal findings are that the local flame structure correlates strongly with the local flame curvature, while global properties depend both on strain and on curvature. Preliminary results for cases with nonhomogeneous reactant mixture strength are reported. Here, the emphasis is on the ability of a propagating flame to recover after encountering a fuel-lean pocket in an otherwise homogeneous mixture. Both one dimensional and two dimensional cases are described.

  4. Lean premixed flames for low NO{sub x} combustors

    SciTech Connect

    Sojka, P.; Tseng, L.; Bryjak, J.

    1995-10-01

    Gas turbines are being used throughout the world to generate electricity. Due to increasing fuel costs and environmental concerns, gas turbines must meet stringent performance requirements, demonstrating high thermal efficiencies and low pollutant emissions. In order for U.S. manufactured gas turbines to stay competitive, their NO{sub x} levels must be below 10 ppm and their thermal efficiencies should approach 60%. Current technology is being stretched to achieve these goals. The twin goals of high efficiency and low NO{sub x} emissions require extending the operating range of current gas turbines. Higher efficiency requires operation at higher pressures and temperatures. Lower NO{sub x} emissions requires lower flame temperatures. Lower flame temperatures can be achieved through partially to fully pre-mixed combustion. However, increased performance and lower emissions result in a set of competing goals. In order to achieve a successful compromise between high efficiency and low NO{sub x} emissions, advanced design tools must be developed. One key design tool is a computationally efficient, high pressure, turbulent flow, combustion model capable of predicting pollutant formation in an actual gas turbine. Its development is the goal of this program. Achieving this goal requires completion of three tasks. The first task is to develop a reduced chemical kinetics model describing N{sub O}x formation in natural gas-air systems. The second task is to develop a computationally efficient model that describes turbulence-chemistry interactions. The third task is to incorporate the reduced chemical kinetics and turbulence-chemistry interaction models into a commercially available flow solver and compare its predictions with experimental data obtained under carefully controlled conditions so that the accuracy of model predictions can be evaluated.

  5. Premixed flame flashback in wall boundary layers studied by long-distance micro-PIV

    NASA Astrophysics Data System (ADS)

    Eichler, Christian; Sattelmayer, Thomas

    2012-02-01

    Premixed flame propagation against the main flow direction in wall boundary layers, a situation known as wall flashback, has been studied by long-distance particle image velocimetry with spatial micron resolution (μ-PIV) and simultaneous flame luminescence recordings. Numerical simulations of laminar wall flashback assist the interpretation of the experimental results. Inside a turbulent boundary layer, the flame propagates in discrete flame cusps pointing in upstream direction and showing a well-defined pattern of formation and break-up. In a laminar boundary layer, the leading flame region is smooth and exhibits low curvature. The instantaneous velocity fields reveal a backflow region upstream of the flame during flashback, which is constrained to the leading flame zone. The backflow is caused by an interaction between the pressure increase upstream of the flame and the boundary layer. The flashback limit is controlled by thermal quenching of the flame tip in the backflow region.

  6. Field Effects of Buoyancy on a Premixed Turbulent Flame Studied by Particle Image Velocimetry

    NASA Technical Reports Server (NTRS)

    Cheng, Robert K.

    2003-01-01

    Typical laboratory flames for the scientific investigation of flame/turbulence interactions are prone to buoyancy effects. Buoyancy acts on these open flame systems and provides upstream feedbacks that control the global flame properties as well as local turbulence/flame interactions. Consequently the flame structures, stabilization limits, and turbulent reaction rates are directly or indirectly coupled with buoyancy. The objective of this study is to characterize the differences between premixed turbulent flames pointing upwards (1g), pointing downwards (-1g), and in microgravity (mg). The configuration is an inverted conical flame stabilized by a small cone-shaped bluff body that we call CLEAN Flames (Cone-Stabilized Lean Flames). We use two laser diagnostics to capture the velocity and scalar fields. Particle image velocimetry (PIV) measures the mean and root mean square velocities and planar imaging by the flame fronts method outlines the flame wrinkle topology. The results were obtained under typical conditions of small domestic heating systems such as water heaters, ovens, and furnaces. Significant differences between the 1g and -1g flames point to the need for including buoyancy contributions in theoretical and numerical calculations. In Earth gravity, there is a complex coupling of buoyancy with the turbulent flow and heat release in the flame. An investigation of buoyancy-free flames in microgravity will provide the key to discern gravity contributions. Data obtained in microgravity flames will provide the benchmark for interpreting and analyzing 1g and -1g flame results.

  7. How ''flat'' is the rich premixed flame produced by your McKenna burner?

    SciTech Connect

    Migliorini, F.; De Iuliis, S.; Cignoli, F.; Zizak, G.

    2008-05-15

    McKenna burners are widely used in the combustion community for producing ''flat'' premixed flames. These flames are considered as standards for the development and calibration of optical techniques. Rich premixed flames produced by McKenna burners are frequently investigated in order to understand soot formation processes both by optical and by sampling techniques. Measurements are normally performed along the axis of the flames, with a uniform distribution of temperature and species concentration assumed in the radial direction. In this work it is shown that the soot radial profiles of rich premixed ethylene-air flames produced by a McKenna burner with a stainless steel porous plug may be far from being ''flat.'' Soot is mainly distributed in an annular region and nonsoot fluorescing species are present in the core of the flames. This surprising result was verified under several working conditions. Furthermore, flames cannot be considered axial-symmetric but present a skewed soot distribution. Another McKenna burner with a bronze porous disk was used to produce flames of the same equivalence ratio and flows. These flames show a completely different soot radial profile, closer to the claimed flat distribution. These results cast doubts about the conclusions drawn in several studies on soot formation performed with a stainless steel McKenna burner. (author)

  8. Numerical study of transient evolution of lifted jet flames: partially premixed flame propagation and influence of physical dimensions

    NASA Astrophysics Data System (ADS)

    Chen, Zhi; Ruan, Shaohong; Swaminathan, Nedunchezhian

    2016-07-01

    Three-dimensional (3D) unsteady Reynolds-averaged Navier-Stokes simulations of a spark-ignited turbulent methane/air jet flame evolving from ignition to stabilisation are conducted for different jet velocities. A partially premixed combustion model is used involving a correlated joint probability density function and both premixed and non-premixed combustion mode contributions. The 3D simulation results for the temporal evolution of the flame's leading edge are compared with previous two-dimensional (2D) results and experimental data. The comparison shows that the final stabilised flame lift-off height is well predicted by both 2D and 3D computations. However, the transient evolution of the flame's leading edge computed from 3D simulation agrees reasonably well with experiment, whereas evident discrepancies were found in the previous 2D study. This difference suggests that the third physical dimension plays an important role during the flame transient evolution process. The flame brush's leading edge displacement speed resulting from reaction, normal and tangential diffusion processes are studied at different typical stages after ignition in order to understand the effect of the third physical dimension further. Substantial differences are found for the reaction and normal diffusion components between 2D and 3D simulations especially in the initial propagation stage. The evolution of reaction progress variable scalar gradients and its interaction with the flow and mixing field in the 3D physical space have an important effect on the flame's leading edge propagation.

  9. Numerical simulation of pollutant emission and flame extinction in lean premixed systems

    NASA Astrophysics Data System (ADS)

    Eggenspieler, Gilles

    Premixed and partially-premixed combustion and pollutant emissions in full-scale gas turbines has been numerically investigated using a massively-parallel Large-Eddy Simulation Combustion Dynamics Model. Through the use of a flamelet library approach, it was observed that CO (Carbon Oxide) and NO (Nitric Oxide) emission can be predicted and match experimental results. The prediction of the CO emission trend is shown to be possible if the influence of the formation of UHC (Unburnt HydroCarbons) via flame extinction is taken into account. Simulations were repeated with two different combustion approach: the G-equation model and the Linear-Eddy Mixing (LEM) Model. Results are similar for these two set of numerical simulations. The LEM model was used to simulate flame extinction and flame lift-off in a dump combustion chamber. The LEM model is compared to the G-equation model and it was found that the LEM model is more versatile than the G-equation model with regard to accurate simulation of flame propagation in all turbulent premixed combustion regimes. With the addition of heat losses, flame extinction was observed for low equivalence ratio. Numerical simulation of flame propagation with transient inflow conditions were also carried out and demonstrated the ability of the LEM model to accurately simulate flame propagation in the case of a partially-premixed system. In all simulations where flame extinction and flame lift-off was simulated, release of unburnt fuel in the post-flame region through flame extinction was not observed.

  10. Subfilter scale combustion modelling for large eddy simulation of turbulent premixed flames

    NASA Astrophysics Data System (ADS)

    Shahbazian, Nasim

    Large eddy simulation (LES) is a powerful computational tool for modelling turbulent combustion processes. However, for reactive flows, LES is still under significant development. In particular, for turbulent premixed flames, a considerable complication of LES is that the flame thickness is generally much smaller than the LES filter width such that the flame front and chemical reactions cannot be resolved on the grid. Accurate and robust subfilter-scale (SFS) models of the unresolved turbulence-chemistry interactions are therefore required and studies are needed to evaluate and improve them. In this thesis, a detailed comparison and evaluation of five different SFS models for turbulence-chemistry interactions in LES of premixed flames is presented. These approaches include both flamelet- and non-flamelet-based models, coupled with simple or tabulated chemistry. The modelling approaches considered herein are: algebraic- and transport-equation variants of the flame surface density (FSD) model, the presumed conditional moment (PCM) with flame prolongation of intrinsic low-dimensional manifold (FPI) tabulated chemistry, or PCM-FPI approach, evaluated with two different presumed probability density function (PDF) models; and conditional source-term estimation (CSE) approach. The predicted LES solutions are compared to the existing laboratory-scale experimental observation of Bunsen-type turbulent premixed methane-air flames, corresponding to lean and stoichiometric conditions lying from the upper limit of the flamelet regime to well within the thin reaction zones regime of the standard regimes diagram. Direct comparison of different SFS approaches allows investigation of stability and performance of the models, while the weaknesses and strengths of each approach are identified. Evaluation of algebraic and transported FSD models highlights the importance of non-equilibrium transport in turbulent premixed flames. The effect of the PDF type for the reaction progress

  11. Subfilter Scale Combustion Modelling for Large Eddy Simulation of Turbulent Premixed Flames

    NASA Astrophysics Data System (ADS)

    Shahbazian, Nasim

    Large eddy simulation (LES) is a powerful computational tool for modelling turbulent combustion processes. However, for reactive flows, LES is still under significant development. In particular, for turbulent premixed flames, a considerable complication of LES is that the flame thickness is generally much smaller than the LES filter width such that the flame front and chemical reactions cannot be resolved on the grid. Accurate and robust subfilter-scale (SFS) models of the unresolved turbulence-chemistry interactions are therefore required and studies are needed to evaluate and improve them. In this thesis, a detailed comparison and evaluation of five different SFS models for turbulence- chemistry interactions in LES of premixed flames is presented. These approaches include both flamelet- and non-flamelet-based models, coupled with simple or tabulated chemistry. The mod- elling approaches considered herein are: algebraic- and transport-equation variants of the flame surface density (FSD) model, the presumed conditional moment (PCM) with flame prolongation of intrinsic low-dimensional manifold (FPI) tabulated chemistry, or PCM-FPI approach, evaluated with two different presumed probability density function (PDF) models; and conditional source-term estimation (CSE) approach. The predicted LES solutions are compared to the existing laboratory-scale experimental observation of Bunsen-type turbulent premixed methane-air flames, corresponding to lean and stoichiometric conditions lying from the upper limit of the flamelet regime to well within the thin reaction zones regime of the standard regimes diagram. Direct comparison of different SFS approaches allows investigation of stability and performance of the models, while the weaknesses and strengths of each approach are identified. Evaluation of algebraic and transported FSD models highlights the importance of non-equilibrium transport in turbulent premixed flames. The effect of the PDF type for the reaction progress

  12. Effects of Buoyancy on Laminar and Turbulent Premixed V-Flame

    NASA Technical Reports Server (NTRS)

    Cheng, Robert K.; Bedat, Benoit

    1997-01-01

    Turbulent combustion occurs naturally in almost all combustion systems and involves complex dynamic coupling of chemical and fluid mechanical processes. It is considered as one of the most challenging combustion research problems today. Though buoyancy has little effect on power generating systems operating under high pressures (e.g., IC engines and turbines), flames in atmospheric burners and the operation of small to medium furnaces and boilers are profoundly affected by buoyancy. Changes in burner orientation impacts on their blow-off, flash-back and extinction limits, and their range of operation, burning rate, heat transfer, and emissions. Theoretically, buoyancy is often neglected in turbulent combustion models. Yet the modeling results are routinely compared with experiments of open laboratory flames that are obviously affected by buoyancy. This inconsistency is an obstacle to reconciling experiments and theories. Consequently, a fundamental understanding of the coupling between turbulent flames and buoyancy is significant to both turbulent combustion science and applications. The overall effect of buoyancy relates to the dynamic interaction between the flame and its surrounding, i.e., the so-called elliptical problem. The overall flame shape, its flowfield, stability, and mean and local burning rates are dictated by both upstream and downstream boundary conditions. In steady propagating premixed flames, buoyancy affects the products region downstream of the flame zone. These effects are manifested upstream through the mean and fluctuating pressure fields to influence flame stretch and flame wrinkling. Intuitively, the effects buoyancy should diminish with increasing flow momentum. This is the justification for excluding buoyancy in turbulent combustion models that treats high Reynolds number flows. The objectives of our experimental research program is to elucidate flame-buoyancy coupling processes in laminar and turbulent premixed flames, and to

  13. On the Interaction of a Premixed Flame with an Acoustic Disturbance

    NASA Technical Reports Server (NTRS)

    Hood, Caroline; Frendi, Abdelkader

    2005-01-01

    The main objective of this research is to analyze the effect of acoustic disturbances on a premixed flame and determine their role in the onset of combustion instabilities. Computations for the one-dimensional, unsteady combustion of a lean premixed methane-air mixture are performed. An acoustic excitation is introduced in the chamber and interacts with the flame front. Our results indicate that as the amplitude of the acoustic excitation is increased, the flame front position fluctuates rapidly. This phenomenon is even more intense when the frequency of the acoustic disturbance matches the fundamental frequency of the chamber. Our results suggest that the interactions between the flame and the acoustic excitation may result in flame extinguishment. In addition various passive control devices are tested and we found that the Helmholtz resonator with rounded inlet corners is the most efficient.

  14. Analysis of the flamelet concept in the numerical simulation of laminar partially premixed flames

    SciTech Connect

    Consul, R.; Oliva, A.; Perez-Segarra, C.D.; Carbonell, D.; de Goey, L.P.H.

    2008-04-15

    The aim of this work is to analyze the application of flamelet models based on the mixture fraction variable and its dissipation rate to the numerical simulation of partially premixed flames. Although the main application of these models is the computation of turbulent flames, this work focuses on the performance of flamelet concept in laminar flame simulations removing, in this way, turbulence closure interactions. A well-known coflow methane/air laminar flame is selected. Five levels of premixing are taken into account from an equivalence ratio {phi}={infinity} (nonpremixed) to {phi}=2.464. Results obtained using the flamelet approaches are compared to data obtained from the detailed solution of the complete transport equations using primitive variables. Numerical simulations of a counterflow flame are also presented to support the discussion of the results. Special emphasis is given to the analysis of the scalar dissipation rate modeling. (author)

  15. Radiation extinction limit of counterflow premixed lean methane-air flames

    SciTech Connect

    Guo, H.; Ju, Y.; Maruta, Kaoru; Niioka, Takashi; Liu, F.

    1997-06-01

    The application of the laminar flamelet concept to turbulent flame modeling requires a detailed understanding of stretched laminar flames. In this study, the authors used numerical methods, including arc-length continuation, to simulate the extinction characteristics of counterflow premixed fuel-lean, methane-air flames. Attention was primarily paid to the effect of radiative heat loss on the extinction characteristics of these flames. The results show that at medium to low values of the stretch rate, the radiative heat loss has a particularly strong impact on the counterflow premixed fuel-lean, methane-air flames. It was also found that, in addition to the stretch extinction limit at a high stretch rate, there exists a radiation extinction limit at a low stretch rate. Furthermore, the relationship between these two extinction limits and the equivalence ratio is obtained.

  16. Flame-vortex interaction and mixing behaviors of turbulent non-premixed jet flames under acoustic forcing

    SciTech Connect

    Kim, Munki; Choi, Youngil; Oh, Jeongseog; Yoon, Youngbin

    2009-12-15

    This study examines the effect of acoustic excitation using forced coaxial air on the flame characteristics of turbulent hydrogen non-premixed flames. A resonance frequency was selected to acoustically excite the coaxial air jet due to its ability to effectively amplify the acoustic amplitude and reduce flame length and NO{sub x} emissions. Acoustic excitation causes the flame length to decrease by 15% and consequently, a 25% reduction in EINO{sub x} is achieved, compared to coaxial air flames without acoustic excitation at the same coaxial air to fuel velocity ratio. Moreover, acoustic excitation induces periodical fluctuation of the coaxial air velocity, thus resulting in slight fluctuation of the fuel velocity. From phase-lock PIV and OH PLIF measurement, the local flow properties at the flame surface were investigated under acoustic forcing. During flame-vortex interaction in the near field region, the entrainment velocity and the flame surface area increased locally near the vortex. This increase in flame surface area and entrainment velocity is believed to be a crucial factor in reducing flame length and NO{sub x} emission in coaxial jet flames with acoustic excitation. Local flame extinction occurred frequently when subjected to an excessive strain rate, indicating that intense mass transfer of fuel and air occurs radially inward at the flame surface. (author)

  17. Nonlinear hydrodynamic and thermoacoustic oscillations of a bluff-body stabilised turbulent premixed flame

    NASA Astrophysics Data System (ADS)

    Lee, Chin Yik; Li, Larry Kin Bong; Juniper, Matthew P.; Cant, Robert Stewart

    2016-01-01

    Turbulent premixed flames often experience thermoacoustic instabilities when the combustion heat release rate is in phase with acoustic pressure fluctuations. Linear methods often assume a priori that oscillations are periodic and occur at a dominant frequency with a fixed amplitude. Such assumptions are not made when using nonlinear analysis. When an oscillation is fully saturated, nonlinear analysis can serve as a useful avenue to reveal flame behaviour far more elaborate than period-one limit cycles, including quasi-periodicity and chaos in hydrodynamically or thermoacoustically self-excited system. In this paper, the behaviour of a bluff-body stabilised turbulent premixed propane/air flame in a model jet-engine afterburner configuration is investigated using computational fluid dynamics. For the frequencies of interest in this investigation, an unsteady Reynolds-averaged Navier-Stokes approach is found to be appropriate. Combustion is represented using a modified laminar flamelet approach with an algebraic closure for the flame surface density. The results are validated by comparison with existing experimental data and with large eddy simulation, and the observed self-excited oscillations in pressure and heat release are studied using methods derived from dynamical systems theory. A systematic analysis is carried out by increasing the equivalence ratio of the reactant stream supplied to the premixed flame. A strong variation in the global flame structure is observed. The flame exhibits a self-excited hydrodynamic oscillation at low equivalence ratios, becomes steady as the equivalence ratio is increased to intermediate values, and again exhibits a self-excited thermoacoustic oscillation at higher equivalence ratios. Rich nonlinear behaviour is observed and the investigation demonstrates that turbulent premixed flames can exhibit complex dynamical behaviour including quasiperiodicity, limit cycles and period-two limit cycles due to the interactions of various

  18. Bluff-body stabilized flame dynamics of lean premixed syngas combustion

    NASA Astrophysics Data System (ADS)

    Im, Hong G.; Kim, Yu Jeong; Lee, Bok Jik; Kaust Team

    2015-11-01

    Recently, syngas combustion has been actively investigated for the potential application to integrated gasification combined cycle (IGCC) systems. While lean premixed combustion is attractive for both reduced emission and enhanced efficiency, flame instability becomes often an issue. Bluff-bodies have been adopted as effective flame holders for practical application of premixed flames. In the present study, high-fidelity direct numerical simulations are conducted to investigate the dynamics of lean premixed syngas flames stabilized on a bluff-body, in particular at the near blow-off regime of the flame. A two-dimensional domain of 4 mm height and 20 mm length with a flame holder of a 1 mm-by-1 mm square geometry is used. For a syngas mixture with the equivalence ratio of 0.5 and the CO:H2 ratio of 1, several distinct flame modes are identified as the inflow velocity approaches to the blowoff limit. The sequences of extinction pathway and combustion characteristics are discussed.

  19. The evolution equation for the flame surface density in turbulent premixed combustion

    NASA Technical Reports Server (NTRS)

    Trouve, Arnaud

    1993-01-01

    The mean reaction rate in flamelet models for turbulent premixed combustion depends on two basic quantities: a mean chemical rate, called the flamelet speed, and the flame surface density. Our previous work had been primarily focused on the problem of the structure and topology of turbulent premixed flames, and it was then determined that the flamelet speed, when space-averaged, is only weakly sensitive to the turbulent flow field. Consequently, the flame surface density is the key quantity that conveys most of the effects of the turbulence on the rate of energy release. In flamelet models, this quantity is obtained via a modeled transport equation called the Sigma-equation. Past theoretical work has produced a rigorous approach that leads to an exact but unclosed formulation for the turbulent Sigma-equation. In the exact Sigma-equation, it appears that the dynamical properties of the flame surface density are determined by a single parameter, namely the turbulent flame stretch. Unfortunately, the turbulent flame stretch as well as the flame surface density is not available from experiments, and, in the absence of experimental data, little is known on the validity of the closure assumptions used in current flamelet models. Direct Numerical Simulation (DNS) is the alternative approach to get basic information on these fundamental quantities. In the present work, three-dimensional DNS of premixed flames in isotropic turbulent flow is used to estimate the different terms appearing in the Sigma-equation. A new methodology is proposed to provide the source and sink terms for the flame surface density, resolved both temporally and spatially throughout the turbulent flame brush. Using this methodology, our objective is to extract the turbulent flame stretch from the DNS data base and then perform extensive comparisons with flamelet models. Thanks to the detailed information produced by the DNS-based analysis, it is expected that this type of comparison will not only

  20. Effects of Buoyancy on the Flowfields of Lean Premixed Turbulent V-Flames

    NASA Technical Reports Server (NTRS)

    Cheng, R. K.; Bedat, B.; Yegian, D. T.; Greenberg, P.

    1999-01-01

    Open laboratory turbulent flames used for investigating fundamental flame turbulence interactions are greatly affected by buoyancy. Though much of our current knowledge is based on observations made in open flames, buoyancy effects are usually not considered in data interpretation, numerical analysis or theories. This inconsistency remains an obstacle to merging experimental observations and theoretical predictions. To better understanding the effects of buoyancy, our research focuses on steady lean premixed flames propagating in fully developed turbulence. We hypothesize that the most significant role of buoyancy forces on these flames is to influence their flowfields through a coupling with the mean and the fluctuating pressure fields. This coupling relates to the elliptical problem that emphasizes the importance of the upstream, wall and downstream boundary conditions in determining all aspects of flame propagation. Therefore, buoyancy has the same significance as other parameters such as flow configuration, and flame geometry.

  1. Effects of operating pressure on flame oscillation and emission characteristics in a partially premixed swirl combustor

    SciTech Connect

    Kim, Jong-Ryul; Choi, Gyung-Min; Kim, Duck-Jool

    2011-01-15

    The influence of varying combustor pressure on flame oscillation and emission characteristics in the partially premixed turbulent flame were investigated. In order to investigate combustion characteristics in the partially premixed turbulent flame, the combustor pressure was controlled in the range of -30 to 30 kPa for each equivalence ratio ({phi} = 0.8-1.2). The r.m.s. of the pressure fluctuations increased with decreasing combustor pressure for the lean condition. The combustor pressure had a sizeable influence on combustion oscillation, whose dominant frequency varied with the combustor pressure. Combustion instabilities could be controlled by increasing the turbulent intensity of the unburned mixture under the lean condition. An unstable flame was caused by incomplete combustion; hence, EICO greatly increased. Furthermore, EINO{sub x} simply reduced with decreasing combustor pressure at a rate of 0.035 g/10 kPa. The possibility of combustion control on the combusting mode and exhaust gas emission was demonstrated. (author)

  2. Study of Turbulent Premixed Flame Propagation using a Laminar Flamelet Model

    NASA Technical Reports Server (NTRS)

    Im, H. G.

    1995-01-01

    The laminar flamelet concept in turbulent reacting flows is considered applicable to many practical combustion systems (Linan & Williams 1993). For turbulent premixed combustion, the laminar flamelet regime is valid when turbulent Karlovitz number is less than unity, which is equivalent to stating that the characteristic thickness of the flame is less than that of a Kolmogorov eddy; this is known as the Klimov-Williams criterion (Williams 1985). In such a case, the flame maintains its laminar structure, and the effect of turbulent flow is merely to wrinkle and strain the flame front. The propagating wrinkled premixed flame can then be described as an infinitesimally thin surface dividing the unburnt fresh mixture and the burnt product.

  3. Mechanisms of combustion limits in premixed gas flames at microgravity

    NASA Technical Reports Server (NTRS)

    Ronney, Paul D.

    1991-01-01

    A three-year experimental and theoretical research program on the mechanisms of combustion limits of premixed gasflames at microgravity was conducted. Progress during this program is identified and avenues for future studies are discussed.

  4. Gravitational Influences on Flame Propagation through Non-Uniform, Premixed Gas Systems

    NASA Technical Reports Server (NTRS)

    Miller, Fletcher J.; Easton, John; Ross, Howard D.; Marchese, Anthony; Perry, David; Kulis, Michael

    2001-01-01

    Flame propagation through non-uniformly premixed (or layered) gases has importance both in useful combustion systems and in unintentional fires. As summarized previously, non-uniform premixed gas combustion receives scant attention compared to the more usual limiting cases of diffusion or uniformly premixed flames, especially regarding the role gravity plays. This paper summarizes our progress on furthering the knowledge of layered combustion, in which a fuel concentration gradient exists normal to the direction of flame spread. We present experimental and numerical results for flame spread through propanol-air layers formed near the flash point temperature (25 C) or near the stoichiometric temperature (33 C). Both the model and experimental results show that the removal of gravity results in a faster spreading flame, by as much as 80% depending on conditions. This is exactly the opposite effect as that predicted by an earlier model reported. We also found that having a gallery lid results in faster flame spread, an effect more pronounced at normal gravity, demonstrating the importance of enclosure geometry. Also reported here is the beginning of our spectroscopic measurements of fuel vapor.

  5. Gravitational Influences on Flame Propagation Through Non-Uniform, Premixed Gas Systems

    NASA Technical Reports Server (NTRS)

    Miller, Fletcher J.; Easton, John; Marchese, Anthony; Hovermann, Fred

    2003-01-01

    Flame propagation through non-uniformly premixed (or layered) gases has importance both in useful combustion systems and in unintentional fires. As summarized recently and in previous Microgravity Workshop papers, non-uniform premixed gas combustion receives scant attention compared to the more usual limiting cases of diffusion or uniformly premixed flames, especially regarding the role gravity plays. This paper summarizes our recent findings on gravitational effects on layered combustion along a floor, in which the fuel concentration gradient exists normal to the direction of flame spread. In an effort to understand the mechanism by which the flames spread faster in microgravity (and much faster, in laboratory coordinates, than the laminar burning velocity for uniform mixtures), we have begun making pressure measurements across the spreading flame front that are described here. Earlier researchers, testing in 1g, claimed that hydrostatic pressure differences could account for the rapid spread rates. Additionally, we present the development of a new apparatus to study flame spread in free (i.e., far from walls), non-homogeneous fuel layers formed in a flow tunnel behind an airfoil that has been tested in normal gravity.

  6. A simulation of a bluff-body stabilized turbulent premixed flame using LES-PDF

    NASA Astrophysics Data System (ADS)

    Kim, Jeonglae; Pope, Stephen

    2013-11-01

    A turbulent premixed flame stabilized by a triangular cylinder as a flame-holder is simulated. The computational condition matches the Volvo experiments (Sjunnesson et al. 1992). Propane is premixed at a fuel lean condition of ϕ = 0 . 65 . For this reactive simulation, LES-PDF formulation is used, similar to Yang et al. (2012). The evolution of Lagrangian particles is simulated by solving stochastic differential equations modeling transport of the composition PDF. Mixing is modeled by the modified IEM model (Viswanathan et al. 2011). Chemical reactions are calculated by ISAT and for the good load balancing, PURAN distribution of ISAT tables is applied (Hiremath et al. 2012). To calculate resolved density, the two-way coupling (Popov & Pope 2013) is applied, solving a transport equation of resolved specific volume to reduce statistical noise. A baseline calculation shows a good agreement with the experimental measurements in turbulence statistics, temperature, and minor species mass fractions. Chemical reaction does not significantly contribute to the overall computational cost, in contrast to non-premixed flame simulations (Hiremath et al. 2013), presumably due to the restricted manifold of the purely premixed flame in the composition space.

  7. Effect of vorticity flip-over on the premixed flame structure: Experimental observation of type-I inflection flames.

    PubMed

    El-Rabii, Hazem; Kazakov, Kirill A

    2015-12-01

    Premixed flames propagating in horizontal tubes are observed to take on a convex shape towards the fresh mixture, which is commonly explained as a buoyancy effect. A recent rigorous analysis has shown, on the contrary, that this process is driven by the balance of vorticity generated by a curved flame front with the baroclinic vorticity, and predicted existence of a regime in which the leading edge of the flame front is concave. We report experimental realization of this regime. Our experiments on ethane and n-butane mixtures with air show that flames with an inflection point on the front are regularly produced in lean mixtures, provided that a sufficiently weak ignition is used. The observed flame shape perfectly agrees with that theoretically predicted. PMID:26764801

  8. Effect of vorticity flip-over on the premixed flame structure: Experimental observation of type-I inflection flames

    NASA Astrophysics Data System (ADS)

    El-Rabii, Hazem; Kazakov, Kirill A.

    2015-12-01

    Premixed flames propagating in horizontal tubes are observed to take on a convex shape towards the fresh mixture, which is commonly explained as a buoyancy effect. A recent rigorous analysis has shown, on the contrary, that this process is driven by the balance of vorticity generated by a curved flame front with the baroclinic vorticity, and predicted existence of a regime in which the leading edge of the flame front is concave. We report experimental realization of this regime. Our experiments on ethane and n -butane mixtures with air show that flames with an inflection point on the front are regularly produced in lean mixtures, provided that a sufficiently weak ignition is used. The observed flame shape perfectly agrees with that theoretically predicted.

  9. Understanding and predicting soot generation in turbulent non-premixed jet flames.

    SciTech Connect

    Wang, Hai; Kook, Sanghoon; Doom, Jeffrey; Oefelein, Joseph Charles; Zhang, Jiayao; Shaddix, Christopher R.; Schefer, Robert W.; Pickett, Lyle M.

    2010-10-01

    This report documents the results of a project funded by DoD's Strategic Environmental Research and Development Program (SERDP) on the science behind development of predictive models for soot emission from gas turbine engines. Measurements of soot formation were performed in laminar flat premixed flames and turbulent non-premixed jet flames at 1 atm pressure and in turbulent liquid spray flames under representative conditions for takeoff in a gas turbine engine. The laminar flames and open jet flames used both ethylene and a prevaporized JP-8 surrogate fuel composed of n-dodecane and m-xylene. The pressurized turbulent jet flame measurements used the JP-8 surrogate fuel and compared its combustion and sooting characteristics to a world-average JP-8 fuel sample. The pressurized jet flame measurements demonstrated that the surrogate was representative of JP-8, with a somewhat higher tendency to soot formation. The premixed flame measurements revealed that flame temperature has a strong impact on the rate of soot nucleation and particle coagulation, but little sensitivity in the overall trends was found with different fuels. An extensive array of non-intrusive optical and laser-based measurements was performed in turbulent non-premixed jet flames established on specially designed piloted burners. Soot concentration data was collected throughout the flames, together with instantaneous images showing the relationship between soot and the OH radical and soot and PAH. A detailed chemical kinetic mechanism for ethylene combustion, including fuel-rich chemistry and benzene formation steps, was compiled, validated, and reduced. The reduced ethylene mechanism was incorporated into a high-fidelity LES code, together with a moment-based soot model and models for thermal radiation, to evaluate the ability of the chemistry and soot models to predict soot formation in the jet diffusion flame. The LES results highlight the importance of including an optically-thick radiation model

  10. Effects of Buoyancy on the Flowfields of Lean Premixed Turbulent V-Flames

    NASA Technical Reports Server (NTRS)

    Cheng, R. K.; Greenberg, P.; Bedat, B.; Yegian, D. T.

    1999-01-01

    Open laboratory turbulent flames used for investigating fundament flame turbulence interactions are greatly affected by buoyancy. Though much of our current knowledge is based on observations made in these open flames, the effects of buoyancy are usually not included in data interpretation, numerical analysis or theories. This inconsistency remains an obstacle to merging experimental observations and theoretical predictions. To better understanding the effects of buoyancy, our research focuses on steady lean premixed flames propagating in fully developed turbulence. We hypothesize that the most significant role of buoyancy forces on these flames is to influence their flowfields through a coupling with mean and fluctuating pressure fields. Changes in flow pattern alter the mean aerodynamic stretch and in turn affect turbulence fluctuation intensities both upstream and downstream of the flame zone. Consequently, flame stabilization, reaction rates, and turbulent flame processes are all affected. This coupling relates to the elliptical problem that emphasizes the importance of the upstream, wall and downstream boundary conditions in determining all aspects of flame propagation. Therefore, buoyancy has the same significance as other parameters such as flow configuration, flame geometry, means of flame stabilization, flame shape, enclosure size, mixture conditions, and flow conditions.

  11. Effects of buoyancy on the flowfields of lean premixed turbulentv-flames

    SciTech Connect

    Cheng, R.K.; Bedat, B.; Yegian, D.T.; Greenberg, P.

    2001-03-01

    Open laboratory turbulent flames used for investigating fundament flame turbulence interactions are greatly affected by buoyancy. Though much of our current knowledge is based on observations made in these open flames, the effects of buoyancy are usually not included in data interpretation, numerical analysis or theories. This inconsistency remains an obstacle to merging experimental observations and theoretical predictions. To better understanding the effects of buoyancy, our research focuses on steady lean premixed flames propagating in fully developed turbulence. We hypothesize that the most significant role of buoyancy forces on these flames is to influence their flowfields through a coupling with mean and fluctuating pressure fields. Changes in flow pattern alter the mean aerodynamic stretch and in turn affect turbulence fluctuation intensities both upstream and downstream of the flame zone. Consequently, flame stabilization, reaction rates, and turbulent flame processes are all affected. This coupling relates to the elliptical problem that emphasizes the importance of the upstream, wall and downstream boundary conditions in determining all aspects of flame propagation. Therefore, buoyancy has the same significance as other parameters such as flow configuration, flame geometry, means of flame stabilization, flame shape, enclosure size, mixture conditions, and flow conditions.

  12. Large eddy simulation and laser diagnostic studies on a low swirl stratified premixed flame

    SciTech Connect

    Nogenmyr, K.-J.; Bai, X.S.; Fureby, C.; Petersson, P.; Collin, R.; Linne, M.

    2008-11-15

    This paper presents numerical simulations and laser diagnostic experiments of a swirling lean premixed methane/air flame with an aim to compare different Large Eddy Simulations (LES) models for reactive flows. An atmospheric-pressure laboratory swirl burner has been developed wherein lean premixed methane/air is injected in an unconfined low-speed flow of air. The flame is stabilized above the burner rim in a moderate swirl flow, triggering weak vortex breakdown in the downstream direction. Both stereoscopic (3-component) PIV and 2-component PIV are used to investigate the flow. Filtered Rayleigh scattering is used to examine the temperature field in the leading flame front. Acetone-Planar Laser Induced Fluorescence (PLIF) is applied to examine the fuel distribution. The experimental data are used to assess two different LES models; one based on level-set G-equation and flamelet chemistry, and the other based on finite rate chemistry with reduced kinetics. The two LES models treat the chemistry differently, which results in different predictions of the flame dynamic behavior and statistics. Yet, great similarity of flame structures was predicted by both models. The LES and experimental data reveal several intrinsic features of the low swirl flame such as the W-shape at the leading front, the highly wrinkled fronts in the shear layers, and the existence of extinction holes in the trailing edge of the flame. The effect of combustion models, the numerical solvers and boundary conditions on the flame and flow predictions was systematically examined. (author)

  13. Large eddy simulation and laser diagnostic studies on a low swirl stratified premixed flame

    SciTech Connect

    Nogenmyr, K.-J.; Bai, X.S.; Fureby, C.; Petersson, P.; Collin, R.; Linne, M.

    2009-01-15

    This paper presents numerical simulations and laser diagnostic experiments of a swirling lean premixed methane/air flame with an aim to compare different Large Eddy Simulations (LES) models for reactive flows. An atmospheric-pressure laboratory swirl burner has been developed wherein lean premixed methane/air is injected in an unconfined low-speed flow of air. The flame is stabilized above the burner rim in a moderate swirl flow, triggering weak vortex breakdown in the downstream direction. Both stereoscopic (3-component) PIV and 2-component PIV are used to investigate the flow. Filtered Rayleigh scattering is used to examine the temperature field in the leading flame front. Acetone-Planar Laser Induced Fluorescence (PLIF) is applied to examine the fuel distribution. The experimental data are used to assess two different LES models; one based on level-set G-equation and flamelet chemistry, and the other based on finite rate chemistry with reduced kinetics. The two LES models treat the chemistry differently, which results in different predictions of the flame dynamic behavior and statistics. Yet, great similarity of flame structures was predicted by both models. The LES and experimental data reveal several intrinsic features of the low swirl flame such as the W-shape at the leading front, the highly wrinkled fronts in the shear layers, and the existence of extinction holes in the trailing edge of the flame. The effect of combustion models, the numerical solvers and boundary conditions on the flame and flow predictions was systematically examined. (author)

  14. An experimental investigation of the interaction between a Karman vortex street and a premixed laminar flame

    NASA Astrophysics Data System (ADS)

    Namer, I.

    1980-12-01

    The interaction of a premixed C2H4-air flame with a Karman vortex street was studied. Laser Doppler anemometry was used for velocity measurements and Rayleigh scattering was used to measure total gas density. A reference hot wire was used to enable phase-locked ensemble averaging to be performed on the data. The velocity measurements for vortex shedding cylinder Reynolds numbers indicated that the vortex street and, hence, the flow field upstream of the flame is deflected by the flame. This is due to the pressure drop across the flame which is necessary to accelerate the flow behind the flame. The vortices were not observed behind the flame. The combination of dilation and increased dissipation consumed the vortices. Density statistics obtained from Rayleigh scattering measurements were compared with predictions by the Bray-Moss-Libby (B-M-L) model which neglects intermediate states. Density fluctuations were overpredicted by the B-M-L model by a small amount.

  15. Propagation of a premixed flame in a divided-chamber combustor

    NASA Technical Reports Server (NTRS)

    Cattolica, R. J.; Barr, P. K.; Mansour, N. N.

    1987-01-01

    The propagation of premixed ethylene-air mixtures (of 0.5, 0.525, 0.55, and 0.65 equivalence ratios) in a divided-chamber combustor was investigated. The vessel, divided by a small cylindrical prechamber, had optical access (for laser-schlieren videography) and was instrumented by a pressure transducer. For the Reynolds numbers of 1870, 2300, and 2830, the observed spatial development of the laminar flames showed that the flame position and shape could be scaled by a characteristic time, based on the burned gas flame speed and the length of the prechamber. Above a Reynolds number of 4330, this scaling breaks down the appearance of Kelvin-Helmholtz instabilities. The observed flame propagation was compared with predictions obtained with a numerical model of flame propagation. The calculated spatial and temporal development of the flame in the main combustion chamber agreed with the experimental observations only for the lowest Reynolds number (1870).

  16. Impact of heat release on strain rate field in turbulent premixed Bunsen flames

    DOE PAGESBeta

    Coriton, Bruno Rene Leon; Frank, Jonathan H.

    2016-08-10

    The effects of combustion on the strain rate field are investigated in turbulent premixed CH4/air Bunsen flames using simultaneous tomographic PIV and OH LIF measurements. Tomographic PIV provides three-dimensional velocity measurements, from which the complete strain rate tensor is determined. The OH LIF measurements are used to determine the position of the flame surface and the flame-normal orientation within the imaging plane. This combination of diagnostic techniques enables quantification of divergence as well as flame-normal and tangential strain rates, which are otherwise biased using only planar measurements. Measurements are compared in three lean-to-stoichiometric flames that have different amounts of heatmore » release and Damköhler numbers greater than unity. The effects of heat release on the principal strain rates and their alignment relative to the local flame normal are analyzed. The extensive strain rate preferentially aligns with the flame normal in the reaction zone, which has been indicated by previous studies. The strength of this alignment increases with increasing heat release and, as a result, the flame-normal strain rate becomes highly extensive. These effects are associated with the gas expansion normal to the flame surface, which is largest for the stoichiometric flame. In the preheat zone, the compressive strain rate has a tendency to align with the flame normal. Away from the flame front, the flame – strain rate alignment is arbitrary in both the reactants and products. The flame-tangential strain rate is on average positive across the flame front, and therefore the turbulent strain rate field contributes to the enhancement of scalar gradients as in passive scalar turbulence. As a result, increases in heat release result in larger positive values of the divergence as well as flame-normal and tangential strain rates, the tangential strain rate has a weaker dependence on heat release than the flame-normal strain rate and the

  17. A numerical investigation of the effects of imperfect premixing on flame propagation

    NASA Astrophysics Data System (ADS)

    Garrido-Lopez, David

    2005-07-01

    Gasoline direct-injection engines and lean-premixed prevaporized combustors have recently emerged as promising technologies for improving combustion efficiency and pollutant emission. In both applications, the time available for the mixing of fuel and oxidizer prior to combustion may be insufficient for the mixture to acquire a homogeneous composition, and this thesis addresses the propagation of premixed flames under such conditions. Previous numerical studies, owing to severe spatio-temporal limitations, have been unable to provide a clear picture of what to expect from the effects of imperfect premixing on turbulent flames, and have not found agreement with existing experimental data. In this study, direct numerical simulations (DNS) of flame propagation in inhomogeneous mixtures with imposed velocity fluctuations are carried out. To avoid aforementioned limitations and to account for important flame dynamics such as the hydrodynamic instability, a configuration that permits larger domains and longer times than previously accessed by DNS is employed. The simulated flows are unavoidably restricted to two dimensions. One-step chemistry and Fick's diffusion law are considered, along with unity Lewis number assumption. It is observed that relatively weak fluctuations in composition alone may lead to a large increase in flame wrinkling and propagation speed, consistent with experimental findings. The hydrodynamic instability caused by gas expansion is found to be responsible for such strong flame response. However, the impact of composition fluctuations diminishes as velocity fluctuations present become more intense, and eventually imperfect premixing ceases to affect the flame brush speed. This effect is explained based on the numerical results, and a criterion for the transition from one regime to the other is provided. It is also found that imperfect premixing always affects the structure of the flame brush. A gradual change in the composition of the unburnt

  18. An experimental and numerical study on the stability and propagation of laminar premixed flames

    NASA Astrophysics Data System (ADS)

    Vagelopoulos, Christina Maria

    The laminar flame speed is a very important property of laminar premixed flames, especially for the validation of chemical kinetics and modeling of turbulent combustion. The counterflow technique is one of the best approaches for the experimental determination of this property because it allows for the establishment of planar, nearly adiabatic, steady, quasi-one dimensional flames that are subjected to well-defined aerodynamic strain rate. However non-linear effects as the strain rate goes to zero lead to overprediction of the laminar flame speed. In the present study these non-linear effects were investigated experimentally and numerically and significant overprediction was verified, particularly for weakly-burning hydrogen/air flames. Subsequently effort was made to establish and study flame properties at a very-low strain rate regime and qualitative and quantitative conclusions were drawn for the stability of the flame surface subjected to very low aerodynamic strain rate, coupled with the effect of gravity and preferential diffusion. A new experimental technique was developed, based on the observation that if a laminar premixed flame undergoes a transition from planar to Bunsen the strain rate changes from positive to negative values and a near-zero strain-rate regime is established. Flame speed measurements were conducted by using LDV for this regime; the flame speed measured is the true laminar flame speed and this is the first time that this property is directly and experimentally measured. Particle Streak velocimetry was developed to evaluate the strain-rates for near-zero strain-rate regime. The laminar flame speed was measured for atmospheric methane/air, ethane/air and propane/air mixtures for the whole range of equivalence ratios; the new data are lower when compared to previous ones and the overprediction is at the order of 15%.

  19. Use of laser-induced ionization to detect soot inception in premixed flames

    NASA Astrophysics Data System (ADS)

    Manzello, Samuel L.; Lee, Eui Ju; Mulholland, George W.

    2005-08-01

    Experimental measurements of laser-induced ionization were performed for ethene-air premixed flames operated near the soot inception point. Soot was ionized with a pulsed laser operated at 532 nm. The ionization signal was collected with a tungsten electrode located in the postflame region. Ionization signals were collected by use of both single-electrode and dual-electrode configurations. Earlier laser-induced- ionization studies focused on the use of a single biased electrode to generate the electric field, with the burner head serving as the path to ground. In many practical combustion systems, a path to ground is not readily available. To apply the laser-induced- ionization diagnostic to these geometries, a dual-electrode geometry must be employed. The influence of electrode configuration, flame equivalence ratio, and flame height on ionization signal detection was determined. The efficacy of the laser-induced-ionization diagnostic in detecting soot inception in the postflame region of a premixed flame by use of a dual-electrode configuration was investigated. Of the dual-electrode configurations tested, the dual-electrode geometry oriented parallel to the laser beam was observed to be most sensitive for detecting the soot inception point in a premixed flame.

  20. Soot Formation in Laminar Premixed Methane/Oxygen Flames at Atmospheric Pressure

    NASA Technical Reports Server (NTRS)

    Xu, F.; Lin, K.-C.; Faeth, G. M.

    1998-01-01

    Flame structure and soot formation were studied within soot-containing laminar premixed mc1hane/oxygen flames at atmospheric pressure. The following measurements were made: soot volume fractions by laser extinction, soot temperatures by multiline emission, gas temperatures (where soot was absent) by corrected fine-wire thermocouples, soot structure by thermophoretic sampling and transmission electron microscope (TEM), major gas species concentrations by sampling and gas chromatography, and gas velocities by laser velocimetry. Present measurements of gas species concentrations were in reasonably good agreement with earlier measurements due to Ramer et al. as well as predictions based on the detailed mechanisms of Frenklach and co-workers and Leung and Lindstedt: the predictions also suggest that H atom concentrations are in local thermodynamic equilibrium throughout the soot formation region. Using this information, it was found that measured soot surface growth rates could be correlated successfully by predictions based on the hydrogen-abstraction/carbon-addition (HACA) mechanisms of both Frenklach and co-workers and Colket and Hall, extending an earlier assessment of these mechanisms for premixed ethylene/air flames to conditions having larger H/C ratios and acetylene concentrations. Measured primary soot particle nucleation rates were somewhat lower than the earlier observations for laminar premixed ethylene/air flames and were significantly lower than corresponding rates in laminar diffusion flames. for reasons that still must be explained.

  1. Soot Formation in Laminar Premixed Methane/Oxygen Flames at Atmospheric Pressure. Appendix H

    NASA Technical Reports Server (NTRS)

    Xu, F.; Lin, K.-C.; Faeth, G. M.; Urban, D. L. (Technical Monitor); Yuan, Z.-G. (Technical Monitor)

    2001-01-01

    Flame structure and soot formation were studied within soot-containing laminar premixed methanefoxygen flames at atmospheric pressure. The following measurements were made: soot volume fractions by laser extinction, soot temperatures by multiline emission, gas temperatures (where soot was absent) by corrected fine-wire thermocouples, soot structure by thermophoretic sampling and transmission electron microscope (TEM), major gas species concentrations by sampling and gas chromatography, and gas velocities by laser velocimetry. Present measurements of gas species concentrations were in reasonably good agreement with earlier measurements due to Ramer et al. as well as predictions based on the detailed mechanisms of Frenklach and co-workers and Leung and Lindstedt; the predictions also suggest that H atom concentrations are in local thermodynamic equilibrium throughout the soot formation region. Using this information, it was found that measured soot surface growth rates could be correlated successfully by predictions based on the hydrogenabstraction/carbon-addition (HACA) mechanisms of both Frenklach and co-workers and Colket and Hall, extending an earlier assessment of these mechanisms for premixed ethylene/air flames to conditions having larger H/C ratios and acetylene concentrations. Measured primary soot particle nucleation rates were somewhat lower than the earlier observations for laminar premixed ethylene/air flames and were significantly lower than corresponding rates in laminar diffusion flames, for reasons that still must be explained.

  2. Use of laser-induced ionization to detect soot inception in premixed flames

    SciTech Connect

    Manzello, Samuel L.; Lee, Eui Ju; Mulholland, George W

    2005-08-20

    Experimental measurements of laser-induced ionization were performed for ethene-air premixed flames operated near the soot inception point. Soot was ionized with a pulsed laser operated at 532 nm. The ionization signal was collected with a tungsten electrode located in the postflame region. Ionization signals were collected by use of both single-electrode and dual-electrode configurations. Earlier laser-induced- ionization studies focused on the use of a single biased electrode to generate the electric field, with the burner head serving as the path to ground. In many practical combustion systems, a path to ground is not readily available. To apply the laser-induced- ionization diagnostic to these geometries, a dual-electrode geometry must be employed. The influence of electrode configuration, flame equivalence ratio, and flame height on ionization signal detection was determined. The efficacy of the laser-induced-ionization diagnostic in detecting soot inception in the postflame region of a premixed flame by use of a dual-electrode configuration was investigated. Of the dual-electrode configurations tested, the dual-electrode geometry oriented parallel to the laser beam was observed to be most sensitive for detecting the soot inception point in a premixed flame.

  3. Subgrid-scale mixing of temperature perturbations from flamelet in turbulent partially premixed flames

    NASA Astrophysics Data System (ADS)

    Liu, Shuaishuai; Tong, Chenning

    2013-11-01

    Recent studies have shown that the subgrid-scale (SGS) mixture fraction and temperature in turbulent partially premixed flames have different structures for different SGS scalar variance. For large SGS variance the molecular transport and chemical reaction are tightly coupled while mixing models are greatly based on non-reactive scalars. To account for this coupling effect we use a method proposed by Bilger and Pope to decompose the temperature (a reactive scalar) into a flamelet part and the perturbations from it. The molecular transport of the former is in close form while the latter in unclosed. The diffusion and dissipation of the temperature perturbations are analyzed using high-resolution line images obtained in turbulent partially premixed (Sandia) flames. The results show that for flame regions that are nearly fully burning, the SGS mixing of the temperature perturbations is similar to that of a non-reactive scalar.

  4. The interaction of water mists and premixed propane-air flames under low-gravity conditions

    NASA Astrophysics Data System (ADS)

    Abbud-Madrid, Angel; Riedel, Edward P.; McKinnon, J. Thomas

    1999-01-01

    A preliminary investigation of the effect of water mists on premixed flame propagation in a cylindrical tube under low-gravity conditions has been conducted to define the scientific and technical objectives of the experiments to be performed on the Space Shuttle and International Space Station microgravity environments. The inhibiting characteristics of water mists in propagating flames of propane-air mixtures at various equivalence ratios are studied. The effects of droplet size and concentration on the laminar flame speed are used as the measure of fire suppression efficacy. Flame speed and propagation behavior are monitored by a video camera. Reduced gravity is obtained with an aircraft flying parabolic trajectories. Measurements and qualitative observations from the low-gravity experiments clearly show the effect of water mist on flame speed abatement, flame shape, and radiant emission. For lean propane-air mixtures, the flame speed increases at first with low water-mist concentrations and then decreases below its dry value when higher water-mist volumes are introduced in the tube. This phenomenon may be due in part to the heating of the unburned mixture ahead of the flame as a result of radiation absorption by the water droplets. For rich propane-air mixtures, similar behavior of flame speed vs. water concentration is encountered but in this case is mostly due to the formation of cellular flames. At high water loads both lean and rich flames exhibit extinction before reaching the end of the tube.

  5. Characteristics of Non-Premixed Turbulent Flames in Microgravity

    NASA Technical Reports Server (NTRS)

    Hegde, U.; Yuan, Z. G.; Stocker, D. P.; Bahadori, M. Y.

    1999-01-01

    The momentum of the fuel (and/or air) jet is important in classifying gas-jet diffusion flame behavior. Normal-gravity data on gas-jet flames show that the flame height (non-dimensionalized with respect to an effective diameter) can be correlated to a density weighted Froude number in the buoyancy-dominated limit. In the momentum-dominated limit this non-dimensional flame height asymptotes to a constant value. The momentum-dominated limit under normal gravity conditions is usually obtained for very high injection velocities which in turn results in high values of the injection Reynolds number. This results in a complicated flame structure because of the large number of turbulence scales involved. In order to gain better insight into the structure of these flames it would be useful to reduce the injection Reynolds number while still maintaining turbulent conditions. This can be done in microgravity where momentum-dominated turbulent flames are obtained at much smaller velocities than in normal gravity. In this paper, experimental results on the effects of nozzle diameter and fuel dilution on flame height are discussed. The experimental values are compared with predictions from a numerical procedure utilizing the standard k-epsilon turbulence model. Flame height scaling with nozzle size and dilution is established. Differences between model predictions and measurements are presented. In order to explain these differences, evolutions of turbulent spectra and Taylor microscale along the flame axis are considered.

  6. Simulations and experiments on the ignition probability in turbulent premixed bluff-body flames

    NASA Astrophysics Data System (ADS)

    Sitte, Michael Philip; Bach, Ellen; Kariuki, James; Bauer, Hans-Jörg; Mastorakos, Epaminondas

    2016-05-01

    The ignition characteristics of a premixed bluff-body burner under lean conditions were investigated experimentally and numerically with a physical model focusing on ignition probability. Visualisation of the flame with a 5 kHz OH* chemiluminescence camera confirmed that successful ignitions were those associated with the movement of the kernel upstream, consistent with previous work on non-premixed systems. Performing many separate ignition trials at the same spark position and flow conditions resulted in a quantification of the ignition probability Pign, which was found to decrease with increasing distance downstream of the bluff body and a decrease in equivalence ratio. Flows corresponding to flames close to the blow-off limit could not be ignited, although such flames were stable if reached from a richer already ignited condition. A detailed comparison with the local Karlovitz number and the mean velocity showed that regions of high Pign are associated with low Ka and negative bulk velocity (i.e. towards the bluff body), although a direct correlation was not possible. A modelling effort that takes convection and localised flame quenching into account by tracking stochastic virtual flame particles, previously validated for non-premixed and spray ignition, was used to estimate the ignition probability. The applicability of this approach to premixed flows was first evaluated by investigating the model's flame propagation mechanism in a uniform turbulence field, which showed that the model reproduces the bending behaviour of the ST-versus-u‧ curve. Then ignition simulations of the bluff-body burner were carried out. The ignition probability map was computed and it was found that the model reproduces all main trends found in the experimental study.

  7. Laser-saturated fluorescence of nitric oxide and chemiluminescence measurements in premixed ethanol flames

    SciTech Connect

    Marques, Carla S.T.; Barreta, Luiz G.; Sbampato, Maria E.; dos Santos, Alberto M.

    2010-11-15

    In this study, nitric oxide laser-saturated fluorescence (LSF) measurements were acquired from premixed ethanol flames at atmospheric pressure in a burner. NO-LSF experimental profiles for fuel-rich premixed ethanol flames ({phi} = 1.34 and {phi} = 1.66) were determined through the excitation/detection scheme of the Q{sub 2}(26.5) rotational line in the A{sup 2}{sigma}{sup +} - X{sup 2}{pi} (0,0) vibronic band and {gamma}(0,1) emission band. A calibration procedure by NO doping into the flame was applied to establish the NO concentration profiles in these flames. Chemiluminescent emission measurements in the (0, 0) vibronic emission bands of the OH{sup *} (A{sup 2}{sigma}{sup +} - X{sup 2}{pi}) and CH{sup *}(A{sup 2}{delta} - X{sup 2}{pi}) radicals were also obtained with high spatial and spectral resolution for fuel-rich premixed ethanol flames to correlate them with NO concentrations. Experimental chemiluminescence profiles and the ratios of the integrated areas under emission spectra (A{sub CH*}/A{sub CH*}(max.) and A{sub CH*}/A{sub OH*}) were determined. The relationships between chemiluminescence and NO concentrations were established along the premixed ethanol flames. There was a strong connection between CH{sup *} radical chemiluminescence and NO formation and the prompt-NO was identified as the governing mechanism for NO production. The results suggest the optimum ratio of the chemiluminescence of two radicals (A{sub CH*}/A{sub OH*}) for NO diagnostic purposes. (author)

  8. Measurements and Modeling of Nitric Oxide Formation in Counterflow, Premixed CH4/O2/N2 Flames

    NASA Technical Reports Server (NTRS)

    Thomsen, D. Douglas; Laurendeau, Normand M.

    2000-01-01

    Laser-induced fluorescence (LIF) measurements of NO concentration in a variety of CH4/O2/N2 flames are used to evaluate the chemical kinetics of NO formation. The analysis begins with previous measurements in flat, laminar, premixed CH4/O2/N2 flames stabilized on a water-cooled McKenna burner at pressures ranging from 1 to 14.6 atm, equivalence ratios from 0.5 to 1.6, and volumetric nitrogen/oxygen dilution ratios of 2.2, 3.1 and 3.76. These measured results are compared to predictions to determine the capabilities and limitations of the comprehensive kinetic mechanism developed by the Gas Research Institute (GRI), version 2.11. The model is shown to predict well the qualitative trends of NO formation in lean-premixed flames, while quantitatively underpredicting NO concentration by 30-50%. For rich flames, the model is unable to even qualitatively match the experimental results. These flames were found to be limited by low temperatures and an inability to separate the flame from the burner surface. In response to these limitations, a counterflow burner was designed for use in opposed premixed flame studies. A new LIF calibration technique was developed and applied to obtain quantitative measurements of NO concentration in laminar, counterflow premixed, CH4/O2/N2 flames at pressures ranging from 1 to 5.1 atm, equivalence ratios of 0.6 to 1.5, and an N2/O2 dilution ratio of 3.76. The counterflow premixed flame measurements are combined with measurements in burner-stabilized premixed flames and counterflow diffusion flames to build a comprehensive database for analysis of the GRI kinetic mechanism. Pathways, quantitative reaction path and sensitivity analyses are applied to the GRI mechanism for these flame conditions. The prompt NO mechanism is found to severely underpredict the amount of NO formed in rich premixed and nitrogen-diluted diffusion flames. This underprediction is traced to uncertainties in the CH kinetics as well as in the nitrogen oxidation chemistry

  9. Occurrence and characterization of carbon nanoparticles below the soot laden zone of a partially premixed flame

    SciTech Connect

    Paul, Bireswar; Datta, Amitava; Datta, Aparna; Saha, Abhijit

    2009-12-15

    An experimental study has been performed to detect the occurrence of nanosized carbon particulates below the soot laden zone of a co-flowing partially premixed flame. Samples have been extracted from different points across the flame and passed through DI water. Absorption and fluorescence spectroscopies have been performed with the collected water suspensions. The occurrence of carbon nanoparticles is evident across the inner flame front. In addition, evidence of naphthalene has also been found inside the inner rich premixed flame. The concentration of naphthalene decreases while that of the carbon nanoparticles increases as the inner flame front is reached. The stability of the nanoparticles in the sample has been ensured by observing that the change in fluorescence quantum yield from the sample over a long duration is small. The band gap energy has been evaluated using the absorption data to characterize the likely structures of the particles in the collected suspension. Two kinds of particles having different zones of band gap energy are found in the flame. Dynamic light scattering measurements show that the particle size grows with the increase in height in the lower part of the flame. While, at 3 and 6 mm elevations the particles are observed to be below 2.5 nm in diameter, the particles at 10 mm elevation are found in the size range of 2.5-5.5 nm. (author)

  10. Local curvature measurements of a lean, partially premixed swirl-stabilised flame

    NASA Astrophysics Data System (ADS)

    Bayley, Alan E.; Hardalupas, Yannis; Taylor, Alex M. K. P.

    2012-04-01

    A swirl-stabilised, lean, partially premixed combustor operating at atmospheric conditions has been used to investigate the local curvature distributions in lifted, stable and thermoacoustically oscillating CH4-air partially premixed flames for bulk cold-flow Reynolds numbers of 15,000 and 23,000. Single-shot OH planar laser-induced fluorescence has been used to capture instantaneous images of these three different flame types. Use of binary thresholding to identify the reactant and product regions in the OH planar laser-induced fluorescence images, in order to extract accurate flame-front locations, is shown to be unsatisfactory for the examined flames. The Canny-Deriche edge detection filter has also been examined and is seen to still leave an unacceptable quantity of artificial flame-fronts. A novel approach has been developed for image analysis where a combination of a non-linear diffusion filter, Sobel gradient and threshold-based curve elimination routines have been used to extract traces of the flame-front to obtain local curvature distributions. A visual comparison of the effectiveness of flame-front identification is made between the novel approach, the threshold binarisation filter and the Canny-Deriche filter. The novel approach appears to most accurately identify the flame-fronts. Example histograms of the curvature for six flame conditions and of the total image area are presented and are found to have a broader range of local flame curvatures for increasing bulk Reynolds numbers. Significantly positive values of mean curvature and marginally positive values of skewness of the histogram have been measured for one lifted flame case, but this is generally accounted for by the effect of flame brush curvature. The mean local flame-front curvature reduces with increasing axial distance from the burner exit plane for all flame types. These changes are more pronounced in the lifted flames but are marginal for the thermoacoustically oscillating flames. It is

  11. Dynamics of premixed flames in a narrow channel with a step-wise wall temperature

    SciTech Connect

    Kurdyumov, Vadim N.; Pizza, Gianmarco; Frouzakis, Christos E.; Mantzaras, John

    2009-11-15

    The effect of channel height, inflow velocity and wall temperature on the dynamics and stability of unity Lewis number premixed flames in channels with specified wall temperature is investigated with steady and transient numerical simulations using a two-dimensional thermo-diffusive model. The simplified model is capable of capturing many of the transitions and the combustion modes observed experimentally and in direct numerical simulations in micro- and meso-scale channels, and indicates that the thermal flame/wall interaction is the mechanism leading to the observed flame instabilities. Finally, an ad-hoc one-dimensional model based on the flame-sheet approximation is tested in its capacity to reproduce some of the flame dynamics of the two-dimensional thermo-diffusive model. (author)

  12. Spatially distributed flame transfer functions for predicting combustion dynamics in lean premixed gas turbine combustors

    SciTech Connect

    Kim, K.T.; Lee, J.G.; Quay, B.D.; Santavicca, D.A.

    2010-09-15

    The present paper describes a methodology to improve the accuracy of prediction of the eigenfrequencies and growth rates of self-induced instabilities and demonstrates its application to a laboratory-scale, swirl-stabilized, lean-premixed, gas turbine combustor. The influence of the spatial heat release distribution is accounted for using local flame transfer function (FTF) measurements. The two-microphone technique and CH{sup *} chemiluminescence intensity measurements are used to determine the input (inlet velocity perturbation) and the output functions (heat release oscillation), respectively, for the local flame transfer functions. The experimentally determined local flame transfer functions are superposed using the flame transfer function superposition principle, and the result is incorporated into an analytic thermoacoustic model, in order to predict the linear stability characteristics of a given system. Results show that when the flame length is not acoustically compact the model prediction calculated using the local flame transfer functions is better than the prediction made using the global flame transfer function. In the case of a flame in the compact flame regime, accurate predictions of eigenfrequencies and growth rates can be obtained using the global flame transfer function. It was also found that the general response characteristics of the local FTF (gain and phase) are qualitatively the same as those of the global FTF. (author)

  13. An experimental study of the structure of laminar premixed flames of ethanol/methane/oxygen/argon

    PubMed Central

    Tran, L.S.; Glaude, P.A.; Battin-Leclerc, F.

    2013-01-01

    The structures of three laminar premixed stoichiometric flames at low pressure (6.7 kPa): a pure methane flame, a pure ethanol flame and a methane flame doped by 30% of ethanol, have been investigated and compared. The results consist of concentration profiles of methane, ethanol, O2, Ar, CO, CO2, H2O, H2, C2H6, C2H4, C2H2, C3H8, C3H6, p-C3H4, a-C3H4, CH2O, CH3HCO, measured as a function of the height above the burner by probe sampling followed by on-line gas chromatography analyses. Flame temperature profiles have been also obtained using a PtRh (6%)-PtRh (30%) type B thermocouple. The similarities and differences between the three flames were analyzed. The results show that, in these three flames, the concentration of the C2 intermediates is much larger than that of the C3 species. In general, mole fraction of all intermediate species in the pure ethanol flame is the largest, followed by the doped flame, and finally the pure methane flame. PMID:24092946

  14. Appearance and stability of a laminar conical premixed flame subjected to an acoustic perturbation

    SciTech Connect

    Bourehla, A.; Baillot, F.

    1998-08-01

    The paper describes an experimental study of quad-conical premixed air/methane flames vibrating under periodic fluctuations of the upstream flow. The flow field and the flame were characterized by an LDV system and image processing. The flow velocity fluctuations were created by an acoustic perturbation with a frequency between 20 and 1000 Hz and a perturbation intensity, defined as the ratio of the rms amplitude of the flow velocity fluctuations to the mean velocity at the exit of the burner, ranging from 0 to 150%. In the perturbation plane (frequency and intensity), a chart is established that shows the configurations assumed by the flame in response to the acoustic perturbation. Three configurations were studied. The wrinkled flame configuration exhibits a flame with undulations symmetrical about the vertical axis and vibrating at the perturbation frequency. This work completes previous studies. In particular, a critical value of the frequency is found. Above this acoustic amplitudes of deformation are damped at the front, which is unaffected by the wrinkling. The subharmonic flame configuration exhibits a flame whose front oscillates with half the perturbation frequency, symmetrical or not, about the burner centerline. The asymmetrical flame is composed of two half-fronts moving in opposition. This instability on Bunsen burners has never previously been observed or predicted. The chaotic flame configuration characterizes a flame not necessarily attached to the burner that exhibits a disordered geometry that leads to aperiodicity of its motion.

  15. Field Effects of Buoyancy on Lean Premixed Turbulent Flames

    NASA Technical Reports Server (NTRS)

    Cheng, R. K.; Dimalanta, R.; Wernet, M. P.; Greenberg, P. S.

    2001-01-01

    Buoyancy affects the entire flowfield of steady turbulent flames and this aspect of flame buoyancy coupling is largely unexplored by experiments or by theory. Open flames and flames within large confinements are free to expand and interact with the surrounding environment. In addition to fluid and combustion conditions, their aerodynamic flowfields are determined by the flame brush orientation and geometry, wake of the stabilizer, enclosure size, and of course, the gravitational field. Because the flowfield consists mainly of cold reactants (mostly in the nearfield) and hot products (mostly in the farfield), buoyancy effects are manifested in the farfield region. In upward pointing flames, an obvious effect is a favorable axial pressure gradient that accelerates the products thereby increasing the axial aerodynamic stretch rate. Intrinsic to turbulent flows, changes in mean aerodynamic stretch also couple to the fluctuating pressure field. Consequently, buoyancy can influence the turbulence intensities upstream and downstream of the flame. Flame wrinkling process, and heat release rate are also directly affected. This backward coupling mechanism is the so-called elliptic problem. To resolve the field effects of buoyancy would require the solution of three-dimensional non-linear Navier Stokes equations with full specification of the upstream, wall and downstream boundary conditions.

  16. The evolution equation for the flame surface density in turbulent premixed combustion

    NASA Technical Reports Server (NTRS)

    Trouve, A.; Poinsot, T.

    1992-01-01

    One central ingredient in flamelet models for turbulent premixed combustion is the flame surface density. This quantity conveys most of the effects of the turbulence on the rate of energy release and is obtained via a modeled transport equation, called the Sigma-equation. Past theoretical work has produced a rigorous approach that leads to an exact, but unclosed, formulation for the turbulent Sigma-equation. In this exact Sigma-equation, it appears that the dynamical properties of the flame surface density are determined by a single parameter, namely the turbulent flame stretch. Unfortunately, the flame surface density and the turbulent flame stretch are not available from experiments and, in the absence of experimental data, little is known on the validity of the closure assumptions used in current flamelet models. Direct Numerical Simulation (DNS) is the obvious, complementary approach to get basic information on these fundamental quantities. Three-dimensional DNS of premixed flames in isotropic turbulent flow is used to estimate the different terms appearing in the Sigma-equation. A new methodology is proposed to provide the source and sink terms for the flame surface density, resolved both temporally and spatially throughout the turbulent flame brush. Using this methodology, the effects of the Lewis number on the rate of production of flame surface area are described in great detail and meaningful comparisons with flamelet models can be performed. The analysis reveals in particular the tendency of the models to overpredict flame surface dissipation as well as their inability to reproduce variations due to thermo-diffusive phenomena. Thanks to the detailed information produced by a DNS-based analysis, this type of comparison not only underscores the shortcomings of current models but also suggests ways to improve them.

  17. The effect of temperature on soot properties in premixed methane flames

    SciTech Connect

    Alfe, M.; Apicella, B.; Tregrossi, A.; Ciajolo, A.; Rouzaud, J.-N.

    2010-10-15

    The effect of flame temperature on soot properties was studied in premixed methane/oxygen flames burning at a constant mixture composition (C/O = 0.60, {phi} = 2.4) and different cold-gas flow velocities (4 and 5 cm s{sup -1}). Temperature and concentration profiles of stable gases and condensed phases combustion products were measured along the flame axis. It was found that the high flame temperature conditions cause a larger decomposition of methane into hydrogen and C{sub 2}-C{sub 4} hydrocarbons, thereby reducing the formation of benzene and condensed phases including condensed species and soot. Soot properties were studied by UV-Visible absorption spectroscopy, thermogravimetry and H/C elemental analysis. A description of soot nanostructural organization was also performed by means of high-resolution transmission electron microscopy. Different properties and nanostructures were found to develop in the soot, depending on the temperature and on soot aging associated. Soot dehydrogenation occurred to a larger extent in the high flame temperature conditions. As soot dehydrogenates the mass absorption coefficients of soot exhibited an increasing trend along the flame axis. However, mature soot retained a relatively high H/C ratio and low absorption coefficients with respect to other less hydrogenated fuels even in high temperature conditions. This indicates that the aromatization/dehydrogenation of soot in premixed flames is more dependent on the fuel characteristics rather than on the flame temperature. Generally, it was assessed that mature soot produced from diverse hydrocarbon fuels with similar flame temperatures and flame types possess a different chemical composition and structure. To this regard the H/C atomic ratio and mass absorption coefficients appeared to be signatures of soot properties and structural evolution. (author)

  18. Tabulation of complex chemistry based on self-similar behavior of laminar premixed flames

    SciTech Connect

    Ribert, G.; Gicquel, O.; Darabiha, N.; Veynante, D.

    2006-09-15

    Detailed mechanisms describing complex phenomena of combustion chemistry, such as flame propagation or pollutant formation, involve hundreds of species and thousands of elementary reactions and cannot be handled in practical simulations of turbulent combustion. A widely used way to reduce chemistry is to build look-up tables where chemical parameters such as reaction rates and/or species mass fractions are determined from a reduced set of coordinates (ILDM, FPI, or FGM methods). Nevertheless, these tables may require large memory spaces and nonnegligible access times, especially when running on massively parallel computers. In this work, the self-similarity behavior of laminar premixed flames is first put into evidence and then theoretically sustained. This property provides a way to reduce the size of chemical databases, especially for computations on massively parallel machines, under the FPI (flame prolongation of ILDM) framework. The database is reduced to similarity profiles for the species reaction rates (or the species mass fractions), stored together with scaling rules. This new formulation is then implemented in the PREMIX code and numerical simulations of laminar premixed flames successfully compare with full chemistry computation, validating this promising approach. (author)

  19. Premixed Edge-Flames in Spatially-Varying Straining Flows

    NASA Technical Reports Server (NTRS)

    Liu, Jian-Bang; Ronney, Paul D.

    1999-01-01

    Flames subject to temporally and spatially uniform hydrodynamic strain are frequently used to model the local interactions of flame fronts with turbulent flow fields (Williams, 1985; Peters, 1986; Bradley, 1992). The applicability of laminar flamelet models in strongly turbulent flows have been questioned recently (Shay and Ronney, 1998) because in turbulent flows the strain rate (sigma) changes at rates comparable to sigma itself and the scale over which the flame front curvature and sigma changes is comparable to the curvature scale itself. Therefore quasi-static, local models of turbulent strain and curvature effects on laminar flamelets may not be accurate under conditions where the strain and curvature effects are most significant. The purpose of this study is to examine flames in spatially-varying strain and compare their properties to those of uniformly strained flames.

  20. Blowoff behavior of bluff body stabilized flames in vitiated and partially premixed flows

    NASA Astrophysics Data System (ADS)

    Tuttle, Steven G.

    Turbulent flame holding and blowoff characteristics of bluff body stabilized flames were measured in an enclosed rectangular duct with a triangular flame holder in vitiated, premixed and unvitiated, asymmetrically stratified flows. Blowoff stability margins were characterized, with chemiluminescence measurements performed by high-speed imaging to capture flame dynamics during blow off. As the equivalence ratio was decreased, local extinction along the shear layer flames occurred with greater frequency and proximity to the wake stagnation zone. Decreased equivalence ratio resulted in extinction events at the trailing edge of the stagnation zone, where reactants were convected into the recirculation zone and burned. Eventually, increasing reactant dilution of the recirculation zone either increased the ignition time scale or the lowered the strain tolerance of the propagating flames in the flame anchoring region, resulting in lift-off or extinction, and the near field shear layer flames convected to the wake stagnation zone, where they continued to propagate. From there, the flames were convected upstream into the recirculation zone, where they were eventually quenched. Simultaneous PIV and OH PLIF measurements captured the flame edge location and aerodynamic behavior as blowoff was approached. Two-dimensional hydrodynamic stretch alone the flame front and flow field vorticity maps were extracted from the combined PIV/OH PLIF data. The distribution of flame stretch shifted to greater values as the equivalence ratio decreased. Asymmetric fuel distributions, measured with acetone LW, were found to increase the equivalence ratio at blow off from that found with uniformly-fueled flows. This was attributed to the greater wake instability and extinction of the lean-side flames. The asymmetrically fueled flames were more susceptible to thermoacoustic instabilities when the shedding frequency was near an acoustic eigenmode of the exhaust duct, due to the decreased

  1. EXPERIMENTAL AND MODELING STUDY OF PREMIXED LAMINAR FLAMES OF ETHANOL AND METHANE

    PubMed Central

    Tran, Luc-Sy; Glaude, Pierre-Alexandre; Fournet, René; Battin-Leclerc, Frédérique

    2013-01-01

    To better understand the chemistry of the combustion of ethanol, the structure of five low pressure laminar premixed flames has been investigated: a pure methane flame (φ=1), three pure ethanol flames (φ=0.7, 1.0, and 1.3), and an ethanol/methane mixture flames (φ=1). The flames have been stabilized on a burner at a pressure of 6.7 kPa using argon as dilutant, with a gas velocity at the burner of 64.3 cm/s at 333 K. The results consist of mole fraction profiles of 20 species measured as a function of the height above the burner by probe sampling followed by online gas chromatography analyses. A mechanism for the oxidation of ethanol was proposed. The reactions of ethanol and acetaldehyde were updated and include recent theoretical calculations while that of ethenol, dimethyl ether, acetone, and propanal were added in the mechanism. This mechanism was also tested against experimental results available in the literature for laminar burning velocities and laminar premixed flame where ethenol was detected. The main reaction pathways of consumption of ethanol are analyzed. The effect of the branching ratios of reaction C2H5OH+OH→Products+H2O is also discussed. PMID:23712124

  2. Direct spectral/hp element simulation of piloted jet non-premixed flames

    NASA Astrophysics Data System (ADS)

    Nastase, Cristian R.

    2004-11-01

    The spectral/hp element method is used for direct numerical simulation (DNS) of piloted non premixed methane jet flames. This method combines the accuracy of spectral methods with versatility of finite element methods, and allows accurate simulations of complex flows on structured and unstructured grids. Here, the methodology is extended for simulation of multi-species, reactive flows using the discontinuous Galerkin formulation. Parallel computation is performed via MPI standards coupled with a domain decomposition methodology. The overall computational scheme allows for an efficient partitioning of the flow configuration. Tests performed with up to 64 processors show quasi-linear parallel performance and scalability. The flame configurations are similar to the piloted jet non-premixed flame considered at the Combustion Research Facility at the Sandia National Laboratories. For a momentum dominated flame, the simulated results portray many of the features observed experimentally. This pertains to both the spatial and the compositional structures of the flow. For a buoyancy controlled flame (at elevated gravity levels), the results indicate an increase in both the turbulence levels and flow acceleration. Departure from equilibrium, including localized extinction is observed on a significant portion of this flame.

  3. DNS and modeling of the interaction between turbulent premixed flames and walls

    NASA Technical Reports Server (NTRS)

    Poinsot, T. J.; Haworth, D. C.

    1992-01-01

    The interaction between turbulent premixed flames and walls is studied using a two-dimensional full Navier-Stokes solver with simple chemistry. The effects of wall distance on the local and global flame structure are investigated. Quenching distances and maximum wall heat fluxes during quenching are computed in laminar cases and are found to be comparable to experimental and analytical results. For turbulent cases, it is shown that quenching distances and maximum heat fluxes remain of the same order as for laminar flames. Based on simulation results, a 'law-of-the-wall' model is derived to describe the interaction between a turbulent premixed flame and a wall. This model is constructed to provide reasonable behavior of flame surface density near a wall under the assumption that flame-wall interaction takes place at scales smaller than the computational mesh. It can be implemented in conjunction with any of several recent flamelet models based on a modeled surface density equation, with no additional constraints on mesh size or time step.

  4. Direct simulation and modeling of flame-wall interaction for premixed turbulent combustion

    SciTech Connect

    Poinsot, T.J.; Haworth, D.C.; Bruneaux, G. . Inst. de Mecanique des Fluides de Toulouse General Motors Research, Warren, MI Inst. Francais du Petrole, Rueil Malmaison )

    1993-10-01

    The interaction between turbulent premixed flames and walls is studied using a two-dimensional full Navier-Stokes solver with simple chemistry. The effects of wall distance on the local and global flame structure are investigated. Quenching distances and maximum wall heat fluxes during quenching are computed in laminar cases and are found to be comparable to experimental and analytical results. For turbulent cases, it is shown that quenching distances and maximum heat fluxes remain of the same order as for laminar flames. Based on simulation results, a law-of-the-wall'' model is derived to describe the interaction between a turbulent premixed flame and a wall. This model is constructed to provide reasonable behavior of flame surface density near a wall under the assumption that flame -- wall interaction takes place at scales smaller than the computational mesh. It can be implemented in conjunction with any of several recent flamelet models based on a modeled surface density equation, with no additional constraints on mesh size or time step. Preliminary tests of this model are presented for the case of a spark-ignited piston engine.

  5. Pre-mixed flame simulations for non-unity Lewis numbers

    NASA Technical Reports Server (NTRS)

    Rutland, C. J.; Trouve, A.

    1990-01-01

    A principal effect of turbulence on premixed flames in the flamelet region is to wrinkle the flame fronts. For non-unity Lewis numbers (Le), the local flame structure is altered in curved regions. This effect is examined using direct numerical simulations of the three dimensional, constant density, decaying isotropic turbulence with a single step, finite rate chemical reaction. Simulations of Lewis numbers 0.8, 1.0, and 1.2 are compared. The turbulent flame speed, S(sub T), increases as Le decreases. The correlation between S(sub T) and u prime found in previous Le = 1 simulations has a strong Lewis number dependency. The variance of the pdf of the flame curvature increases as Le decreases, indicating that the flames become more wrinkled. A strong correlation between local flame speed and curvature was found. For Le greater than 1, the flame speed increases in regions concave towards the products and decreases in convex regions. The opposite correlation was found for Le less than 1. The mean temperature of the products was also found to vary with Lewis number. For Le = 0.8, it is less than the adiabatic flame temperature and for Le = 1.2 it is greater.

  6. Large-Eddy Simulations of Turbulent Premixed Bunsen Flames at Different Turbulence Levels

    NASA Astrophysics Data System (ADS)

    Duchampde Lageneste, Laurent; Pitsch, Heinz

    2002-11-01

    In a recent study we have formulated a level-set method based on the G-equation for Large-Eddy Simulation (LES) of premixed turbulent combustion and applied the model successfully in a simulation of the turbulent Bunsen flame,F3, experimentally investigated by Chen et al. (1996). This flame is nominally in the thin reaction zones regime. As a further validation of the model and to demonstrate the benefits of LES in turbulent combustion modeling, in the present work, we report on an LES of the F2-flame from the same series of experiments, which has a higher turbulence level and hence a higher Karlovitz number. This flame is still in the thin reaction zones regime, but locally reveals regions burning in the broken reaction zones regime. Results from the simulation will be compared with experimental data for temperature and axial velocity. The experimental data shows substantial differences between flames F2 and F3, which is well described by the simulation. Flame F2, for instance, shows an almost linear increase of the flame brush thickness with downstream distance from the nozzle, whereas flame F3 shows almost constant flame brush thickness.

  7. Direct numerical simulation of non-premixed flame-wall interactions

    NASA Astrophysics Data System (ADS)

    Wang, Y.; Trouvé, A.

    2005-01-01

    The overall objective of this paper is to illustrate how detailed numerical modelling may be used to bring basic information on fundamental problems in combustion science. We consider in the following the interaction of non-premixed flames with cold solid wall surfaces. Flame-wall interactions are an important feature in many combustion systems, that result in significant changes in the flame and wall dynamics: the flame strength is reduced near cold wall surfaces, leading possibly to (partial or total) quenching, while the gassolid heat flux takes peak values at flame contact. The questions of turbulent fuel-air-temperature mixing, flame extinction and wall surface heat transfer are here studied using direct numerical simulation (DNS). The DNS configuration corresponds to an ethylene-air diffusion flame stabilized in the near-wall region of a chemically-inert solid surface. Simulations are performed with adiabatic or isothermal wall boundary conditions, and with different turbulence intensities. The simulations feature flame extinction events resulting from excessive wall cooling, and convective heat transfer up to 90 kW/m2. The structure of the simulated wall flames is studied in terms of a classical mass mixing variable, i.e. the fuel-airbased mixture fraction, and a less familiar heat loss variable, i.e. the excess enthalpy variable, introduced to provide a measure of non-adiabatic behavior due to wall cooling.

  8. A numerical study on propagation of premixed flames in small tubes

    SciTech Connect

    Kim, Nam Il; Maruta, Kaoru

    2006-07-15

    A premixed flame in a tube suffers strong variation in its shape and structure depending on boundary conditions. The effects of thermal boundary conditions and flow fields on flame propagation are numerically investigated. This study employs eight combinations of thermal and velocity boundary conditions. Navier-Stokes equations and species equations are solved with a one-step irreversible global reaction model of methane-air mixtures. Finite volume method using an adaptive grid method is applied to investigate the flame structure. In the case of an adiabatic wall, friction force on the wall significantly affected the flame structure while in the case of an isothermal wall, local quenching near the wall dominated flame shape and propagation. In both cases, variations of flow fields occurred not only in the near field of the flame but also within the flame itself, which affected propagation velocities. Near the quenching conditions, strong similarity in the flame structure was found regardless of the boundary velocity profiles due to self-induced velocity deformation. This study provides an overview of the characteristics of flames in small tubes at a steady state. (author)

  9. Response of flame thickness and propagation speed under intense turbulence in spatially developing lean premixed methane–air jet flames

    DOE PAGESBeta

    Sankaran, Ramanan; Hawkes, Evatt R.; Yoo, Chun Sang; Chen, Jacqueline H.

    2015-06-22

    Direct numerical simulations of three-dimensional spatially-developing turbulent Bunsen flames were performed at three different turbulence intensities. We performed these simulations using a reduced methane–air chemical mechanism which was specifically tailored for the lean premixed conditions simulated here. A planar-jet turbulent Bunsen flame configuration was used in which turbulent preheated methane–air mixture at 0.7 equivalence ratio issued through a central jet and was surrounded by a hot laminar coflow of burned products. The turbulence characteristics at the jet inflow were selected such that combustion occured in the thin reaction zones (TRZ) regime. At the lowest turbulence intensity, the conditions fall onmore » the boundary between the TRZ regime and the corrugated flamelet regime, and progressively moved further into the TRZ regime by increasing the turbulent intensity. The data from the three simulations was analyzed to understand the effect of turbulent stirring on the flame structure and thickness. Furthermore, statistical analysis of the data showed that the thermal preheat layer of the flame was thickened due to the action of turbulence, but the reaction zone was not significantly affected. A global and local analysis of the burning velocity of the flame was performed to compare the different flames. Detailed statistical averages of the flame speed were also obtained to study the spatial dependence of displacement speed and its correlation to strain rate and curvature.« less

  10. Response of flame thickness and propagation speed under intense turbulence in spatially developing lean premixed methane–air jet flames

    SciTech Connect

    Sankaran, Ramanan; Hawkes, Evatt R.; Yoo, Chun Sang; Chen, Jacqueline H.

    2015-06-22

    Direct numerical simulations of three-dimensional spatially-developing turbulent Bunsen flames were performed at three different turbulence intensities. We performed these simulations using a reduced methane–air chemical mechanism which was specifically tailored for the lean premixed conditions simulated here. A planar-jet turbulent Bunsen flame configuration was used in which turbulent preheated methane–air mixture at 0.7 equivalence ratio issued through a central jet and was surrounded by a hot laminar coflow of burned products. The turbulence characteristics at the jet inflow were selected such that combustion occured in the thin reaction zones (TRZ) regime. At the lowest turbulence intensity, the conditions fall on the boundary between the TRZ regime and the corrugated flamelet regime, and progressively moved further into the TRZ regime by increasing the turbulent intensity. The data from the three simulations was analyzed to understand the effect of turbulent stirring on the flame structure and thickness. Furthermore, statistical analysis of the data showed that the thermal preheat layer of the flame was thickened due to the action of turbulence, but the reaction zone was not significantly affected. A global and local analysis of the burning velocity of the flame was performed to compare the different flames. Detailed statistical averages of the flame speed were also obtained to study the spatial dependence of displacement speed and its correlation to strain rate and curvature.

  11. Numerical simulation of thermoacoustic response of laboratory scale premixed multi-slit burner flames

    NASA Astrophysics Data System (ADS)

    O'Brien, Adam

    Thermoacoustic instabilities are an entirely unwanted, yet nearly inevitable phenomenon occurring in many practical premixed combustors. If not properly accounted and designed for, they can incur significant increases in the development combustion systems. The fact that such unexpected issues are encountered is indicative of a fundamental lack of understanding regarding the mechanisms that drive thermoacoustic phenomena. Numerical techniques are used to characterize the thermoacoustic response of premixed multi-slit bunsen burner flames. A symmetrical representation of the multi-slit burner is used, and the transfer function is computed at several different frequencies and at three different equivalence ratios. The numerical results are then compared against experimental results in order to determine the suitability of numerical techniques for studying thermoacoustics. A fully compressible Navier-Stokes combustion solver is used in conjunction with adaptive mesh refinement (AMR) for improved resolution at the flame interface.

  12. Consistent flamelet modeling of differential molecular diffusion for turbulent non-premixed flames

    NASA Astrophysics Data System (ADS)

    Wang, Haifeng

    2016-03-01

    Treating differential molecular diffusion correctly and accurately remains as a great challenge to the modeling of turbulent non-premixed combustion. The aim of this paper is to develop consistent modeling strategies for differential molecular diffusion in flamelet models. Two types of differential molecular diffusion models are introduced, linear differential diffusion models and nonlinear differential diffusion models. A multi-component turbulent mixing layer problem is analyzed in detail to gain insights into differential molecular diffusion and its characteristics, particularly the dependence of differential molecular diffusion on the Reynolds number and the Lewis number. These characteristics are then used to validate the differential molecular diffusion models. Finally, the new models are applied to the modeling of a series of laboratory-scale turbulent non-premixed jet flames with different Reynolds number (Sandia Flames B, C, and D) to further assess the models' performance.

  13. A New Type of Steady and Stable, Laminar, Premixed Flame in Ultra-Lean, Hydrogen-Air Combustion

    SciTech Connect

    Grcar, Joseph F; Grcar, Joseph F

    2008-06-30

    Ultra-lean, hydrogen-air mixtures are found to support another kind of laminar flame that is steady and stable beside flat flames and flame balls. Direct numerical simulations are performed of flames that develop into steadily and stably propagating cells. These cells were the original meaning of the word"flamelet'' when they were observed in lean flammability studies conducted early in the development of combustion science. Several aspects of these two-dimensional flame cells are identified and are contrasted with the properties of one-dimensional flame balls and flat flames. Although lean hydrogen-air flames are subject to thermo-diffusive effects, in this case the result is to stabilize the flame rather than to render it unstable. The flame cells may be useful as basic components of engineering models for premixed combustion when the other types of idealized flames are inapplicable.

  14. Low and High Temperature Combustion Chemistry of Butanol Isomers in Premixed Flames and Autoignition Systems

    SciTech Connect

    Sarathy, S M; Pitz, W J; Westbrook, C K; Mehl, M; Yasunaga, K; Curran, H J; Tsujimura, T; Osswald, P; Kohse-Hoinghaus, K

    2010-12-12

    Butanol is a fuel that has been proposed as a bio-derived alternative to conventional petroleum derived fuels. The structural isomer in traditional 'bio-butanol' fuel is n-butanol, but newer conversion technologies produce iso-butanol as a fuel. In order to better understand the combustion chemistry of bio-butanol, this study presents a comprehensive chemical kinetic model for all the four isomers of butanol (e.g., 1-, 2-, iso- and tert-butanol). The proposed model includes detailed high temperature and low temperature reaction pathways. In this study, the primary experimental validation target for the model is premixed flat low-pressure flame species profiles obtained using molecular beam mass spectrometry (MBMS). The model is also validated against previously published data for premixed flame velocity and n-butanol rapid compression machine and shock tube ignition delay. The agreement with these data sets is reasonably good. The dominant reaction pathways at the various pressures and temperatures studied are elucidated. At low temperature conditions, we found that the reaction of alphahydroxybutyl with O{sub 2} was important in controlling the reactivity of the system, and for correctly predicting C{sub 4} aldehyde profiles in low pressure premixed flames. Enol-keto isomerization reactions assisted by HO{sub 2} were also found to be important in converting enols to aldehydes and ketones in the low pressure premixed flames. In the paper, we describe how the structural features of the four different butanol isomers lead to differences in the combustion properties of each isomer.

  15. On the structure, propagation, and stabilization of laminar premixed flames. Final report

    SciTech Connect

    Law, Chung K.

    1999-07-01

    The primary objective of the funded program was to qualitatively understand and quantitatively determine the structure and dynamics of laminar premixed flames. The investigation was conducted using laser-based experimentation, computational simulation with detailed chemistry and transport, and activation energy asymptotic analysis. Highlights of accomplishments were discussed in the annual reports submitted to the program monitor for this project. Details are reported in the thirty journal publications cited in the journal article list which is the major component of this final report.

  16. Self-organized Spiral and Circular Waves in Premixed Gas Flames

    NASA Technical Reports Server (NTRS)

    Pealman, Howard G.; Ronney, Paul D.

    1994-01-01

    A diffusive-thermal high Lewis number (Le) gas-phase oscillator has been observed in premixed flames using a lean mixture of butane and oxygen diluted with helium (Le approx. 3.0). This reactive-diffusive system exhibits both propagating radial pulsations and rotating spiral waves perhaps,analogous to those observed in other excitable media such as the Belousov-Zhabotinsky reaction.

  17. Self-organized spiral and circular waves in premixed gas flames

    NASA Technical Reports Server (NTRS)

    Pearlman, Howard G.; Ronney, Paul D.

    1994-01-01

    A diffusive-thermal high Lewis number (Le) gas-phase oscillator has been observed in premixed flames using a lean mixture of butane and oxygen diluted with helium (Le approximately equals 3.0). This reactive-diffusive system exhibits both propagating radial pulsations and rotating spiral waves perhaps analogous to those observed in other excitable media such as the Belousov-Zhabotinsky reaction.

  18. Structure of the Soot Growth Region of Laminar Premixer Methane/Oxygen Flames

    NASA Technical Reports Server (NTRS)

    Xu, F.; Faeth, G. M.

    1999-01-01

    Soot is a dominant feature of hydrocarbon/air flames, affecting their reaction mechanisms and structure. As a result, soot processes affect capabilities for computational combustion as well as predictions of flame radiation and pollution emissions. Motivated by these observations, the present investigation extended past work on soot growth in laminar premixed flames, seeking to evaluate model predictions of flame structure. Xu et al. report direct measurements of soot residence times, soot concentrations, soot structure, gas temperatures and gas compositions for premixed flames similar to those studied by Harris and Weiner and Ramer et al. respectively. It was found that predictions of major stable gas species concentrations based on mechanisms of Leung and Lindstedt and Frenklach and coworkers, were in good agreement with the measurements. The results were also used to evaluate the hydrogen-abstraction/carbon-addition (HACA) soot growth mechanisms of Frenklach and coworkers and Colket and Hall. It was found that these mechanisms were effective using quite reasonable correlations for the steric factors appearing in the theories. The successful evaluation of the HACA mechanism of soot growth in Refs. 1 and 2 is encouraging but one aspect of this evaluation is a concern. In particular, H-atom concentrations play a crucial role in the HACA mechanism and it was necessary to estimate these concentrations because they were not measured directly. These estimates were made assuming local thermodynamic equilibrium between H, and H based on measured temperatures and H2 concentrations and the equilibrium constant data of Kee et al.. This approach was justified by the flame structure predictions; nevertheless, direct evaluation of equilibrium estimates of H-atom concentrations in the soot growth regions of laminar premixed flames is needed to provide more convincing proof of this behavior. Thus, the objective of the present investigation was to complete new measurements of the

  19. A comparison of transport algorithms for premixed, laminar steady state flames

    NASA Technical Reports Server (NTRS)

    Coffee, T. P.; Heimerl, J. M.

    1980-01-01

    The effects of different methods of approximating multispecies transport phenomena in models of premixed, laminar, steady state flames were studied. Five approximation methods that span a wide range of computational complexity were developed. Identical data for individual species properties were used for each method. Each approximation method is employed in the numerical solution of a set of five H2-02-N2 flames. For each flame the computed species and temperature profiles, as well as the computed flame speeds, are found to be very nearly independent of the approximation method used. This does not indicate that transport phenomena are unimportant, but rather that the selection of the input values for the individual species transport properties is more important than the selection of the method used to approximate the multispecies transport. Based on these results, a sixth approximation method was developed that is computationally efficient and provides results extremely close to the most sophisticated and precise method used.

  20. Demonstration of a burner for the investigation of partially premixed low-temperature flames

    SciTech Connect

    Struckmeier, U.; Lucassen, A.; Kohse-Hoeinghaus, K.; Hansen, N.; Wada, T.; Peters, N.

    2010-10-15

    A burner, which stabilizes near-one-dimensional low-temperature flames at atmospheric pressure, was designed to access the combustion regime near 1500 K for quantitative species diagnostics. Combustion temperatures between 1300 and 1800 K in argon-diluted methane-oxygen flames were achieved by preheating the burner and adapting the inert gas flow. Mass spectrometry with electron ionization was used to determine mole fractions profiles of reactants, products, and intermediates. Combustion parameters were varied including stoichiometry, diluent mole fraction and preheat temperature. Mole fraction profiles resemble those taken in regular premixed flat flames. A number of C{sub 1}- and C{sub 2}-intermediates as well as some oxygenated species were identified. Higher-mass species (m/z > 42) were not detected in the low-temperature methane-oxygen flames which contain 90% argon in the cold gases. (author)

  1. Linear and non-linear forced response of a conical, ducted, laminar premixed flame

    SciTech Connect

    Karimi, Nader; Brear, Michael J.; Jin, Seong-Ho; Monty, Jason P.

    2009-11-15

    This paper presents an experimental study on the dynamics of a ducted, conical, laminar premixed flame subjected to acoustic excitation of varying amplitudes. The flame transfer function is measured over a range of forcing frequencies and equivalence ratios. In keeping with previous works, the measured flame transfer function is in good agreement with that predicted by linear kinematic theory at low amplitudes of acoustic velocity excitation. However, a systematic departure from linear behaviour is observed as the amplitude of the velocity forcing upstream of the flame increases. This non-linearity is mostly in the phase of the transfer function and manifests itself as a roughly constant phase at high forcing amplitude. Nonetheless, as predicted by non-linear kinematic arguments, the response always remains close to linear at low forcing frequencies, regardless of the forcing amplitude. The origin of this phase behaviour is then sought through optical data post-processing. (author)

  2. The production of premixed flame surface area in turbulent shear flow

    NASA Technical Reports Server (NTRS)

    Trouve, A.

    1993-01-01

    In the present work, we use three-dimensional Direct Numerical Simulation (DNS) of premixed flames in turbulent shear flow to characterize the effect of a mean shear motion on flame surface production. The shear is uniform in the unburnt gas, and simulations are performed for different values of the mean shear rate, S. The data base is then used to estimate and compare the different terms appearing in the Sigma-equation as a function of S. The analysis gives in particular the relative weights f the turbulent flow and mean flow components, a(sub T) and A(sub T), of the flame surface production term. This comparison indicates whether the dominant effects of a mean flow velocity gradient on flame surface area are implicit and scale with the modified turbulent flow parameters, kappa and epsilon, or explicit and scale directly with the rate of deformation.

  3. A comparison of experimental results of soot production in laminar premixed flames

    NASA Astrophysics Data System (ADS)

    Caetano, Nattan R.; Soares, Diego; Nunes, Roger P.; Pereira, Fernando M.; Smith Schneider, Paulo; Vielmo, Horácio A.; van der Laan, Flávio Tadeu

    2015-05-01

    Soot emission has been the focus of numerous studies due to the numerous applications in industry, as well as the harmful effects caused to the environment. Thus, the purpose of this work is to analyze the soot formation in a flat flame burner using premixed compressed natural gas and air, where these quasi-adiabatic flames have one-dimensional characteristics. The measurements were performed applying the light extinction technique. The air/fuel equivalence ratiowas varied to assess the soot volume fractions for different flame configurations. Soot production along the flamewas also analyzed by measurements at different heights in relation to the burner surface. Results indicate that soot volume fraction increases with the equivalence ratio. The higher regions of the flamewere analyzed in order to map the soot distribution on these flames. The results are incorporated into the experimental database for measurement techniques calibration and for computational models validation of soot formation in methane premixed laminar flames, where the equivalence ratio ranging from 1.5 up to 8.

  4. Asymptotic analysis of stationary adiabatic premixed flames in porous inert media

    SciTech Connect

    Pereira, Fernando M.; Oliveira, Amir A.M.; Fachini, Fernando F.

    2009-01-15

    The structure of adiabatic premixed flames within porous inert media is investigated using the asymptotic expansion method. For this, the flame structure is divided into three characteristic length scales. The two innermost length scales, the gas-phase diffusion length scale and the reaction length scale, are the same scales defined in the classical premixed flame structure analysis. The outermost length scale, the solid-phase diffusion length scale, is related to the heat conduction in the porous matrix. The differences among these three characteristic length-scales result in large temperature differences between the phases and justify the application of asymptotic expansions to determine an approximate (analytical) solution. Since the main focus of this work is the examination of the processes in the outer and the first inner regions, the simplest kinetic mechanism of one global step is adopted to represent the fuel and oxygen consumption. Then, the description of the reaction zone is obtained using the large activation energy asymptotic method. The description of the problem of the order of the gas-phase length scale is obtained using the boundary layer expansion. This work evaluates the influence of the equivalence ratio, the ratio of the solid to the gas thermal conductivities, the porosity of the medium and the fuel Lewis number on such flames. A parameter that universalizes the flame properties is then identified and discussed. (author)

  5. Asymptotic analysis of stationary adiabatic premixed flames in porous inert media

    SciTech Connect

    Pereira, Fernando M.; Oliveira, Amir A.M.; Fachini, Fernando F.

    2008-11-15

    The structure of adiabatic premixed flames within porous inert media is investigated using the asymptotic expansion method. For this, the flame structure is divided into three characteristic length scales. The two innermost length scales, the gas-phase diffusion length scale and the reaction length scale, are the same scales defined in the classical premixed flame structure analysis. The outermost length scale, the solid-phase diffusion length scale, is related to the heat conduction in the porous matrix. The differences among these three characteristic length-scales result in large temperature differences between the phases and justify the application of asymptotic expansions to determine an approximate (analytical) solution. Since the main focus of this work is the examination of the processes in the outer and the first inner regions, the simplest kinetic mechanism of one global step is adopted to represent the fuel and oxygen consumption. Then, the description of the reaction zone is obtained using the large activation energy asymptotic method. The description of the problem of the order of the gas-phase length scale is obtained using the boundary layer expansion. This work evaluates the influence of the equivalence ratio, the ratio of the solid to the gas thermal conductivities, the porosity of the medium and the fuel Lewis number on such flames. A parameter that universalizes the flame properties is then identified and discussed. (author)

  6. Effects of Lewis number on vorticity and enstrophy transport in turbulent premixed flames

    NASA Astrophysics Data System (ADS)

    Chakraborty, Nilanjan; Konstantinou, Ilias; Lipatnikov, Andrei

    2016-01-01

    The effects of Lewis number Le on both vorticity and enstrophy transport within the flame brush have been analysed using direct numerical simulation data of freely propagating statistically planar turbulent premixed flames, representing the thin reaction zone regime of premixed turbulent combustion. In the simulations, Le was ranged from 0.34 to 1.2 by keeping the laminar flame speed, thermal thickness, Damköhler, Karlovitz, and Reynolds numbers unchanged. The enstrophy has been shown to decay significantly from the unburned to the burned gas side of the flame brush in the Le ≈ 1.0 flames. However, a considerable amount of enstrophy generation within the flame brush has been observed for the Le = 0.34 case and a similar qualitative behaviour has been observed in a much smaller extent for the Le = 0.6 case. The vorticity components have been shown to exhibit anisotropic behaviour within the flame brush, and the extent of anisotropy increases with decreasing Le. The baroclinic torque term has been shown to be principally responsible for this anisotropic behaviour. The vortex stretching and viscous dissipation terms have been found to be the leading order contributors to the enstrophy transport for all cases, but the baroclinic torque and the sink term due to dilatation play increasingly important role for flames with decreasing Le. Furthermore, the correlation between the fluctuations of enstrophy and dilatation rate has been shown to play an important role in determining the material derivative of enstrophy based on the mean flow in the case of a low Le.

  7. Soot Formation in Laminar Premixed Ethylene/Air Flames at Atmospheric Pressure. Appendix G

    NASA Technical Reports Server (NTRS)

    Xu, F.; Sunderland, P. B.; Faeth, G. M.; Urban, D. L. (Technical Monitor)

    2001-01-01

    Soot formation was studied within laminar premixed ethylene/air flames (C/O ratios of 0.78-0.98) stabilized on a flat-flame burner operating at atmospheric pressure. Measurements included soot volume fractions by both laser extinction and gravimetric methods, temperatures by multiline emission, soot structure by thermophoretic sampling and transmission electron microscopy, major gas species concentrations by sampling and gas chromatography, concentrations of condensable hydrocarbons by gravimetric sampling. and velocities by laser velocimetry. These data were used to find soot surface growth rates and primary soot particle nucleation rates along the axes of the flames. Present measurements of soot surface growth rates were correlated successfully by predictions based on typical hydrogen-abstraction/carbon-addition (HACA) mechanisms of Frenklach and co-workers and Colket and Hall. These results suavest that reduced soot surface growth rates with increasing residence time seen in the present and other similar flames were mainly caused by reduced rates of surface activation due to reduced H atom concentrations as temperatures decrease as a result of radiative heat losses. Primary soot particle nucleation rates exhibited variations with temperature and acetylene concentrations that were similar to recent observations for diffusion flames; however, nucleation rates in the premixed flames were significantly lower than in, the diffusion flames for reasons that still must be explained. Finally, predictions of yields of major gas species based on mechanisms from both Frenklach and co-workers and Leung and Lindstedt were in good agreement with present measurements and suggest that H atom concentrations (relevant to HACA mechanisms) approximate estimates based on local thermodynamic equilibrium in the present flames.

  8. Combustion dynamics linked to flame behaviour in a partially premixed swirled industrial burner

    SciTech Connect

    Biagioli, Fernando; Guethe, Felix; Schuermans, Bruno

    2008-07-15

    Previous work [Biagioli, F., Stabilization mechanism of turbulent premixed flames in strongly swirled flows, Combustion, Theory and Modelling 10 (3) (2006) 389-412; Guethe, F., Lachner, R., Schuermans, B., Biagioli, F., Geng, W., Inauen, A., Schenker, S., Bombach, R., Hubschmid, W., Flame imaging on the ALSTOM EV-burner: thermo acoustic pulsations and CFD-validation, in: AIAA Paper 2006-437 presented at the 44th AIAA Aerospace Sciences Meeting and Exhibit, Reno, Nevada, January 9-12, 2006] has shown that turbulent dry low NO{sub x} (partially premixed) flames in high swirl conical burners may be subject to a large change of their anchoring location at the symmetry axis when a critical value of the bulk equivalence ratio is reached, i.e. they are bi-stable. This flame behavior is linked here to combustion pressure dynamics measured in an atmospheric test rig for a prototype version of the Alstom EnVironmental (EV) conical burner. The link is made via the solution of the problem of the 'travelling flameholder', which shows that the unsteady displacement of the flame anchoring location implies an unsteady variation of the flame surface area and therefore unsteady heat release. The relevance of this source of unsteady heat release - which is different from more usual ones due to variations in turbulent burning rate and in the sensible enthalpy jump across the flame - to the generation of combustion dynamics in strongly swirled flows is confirmed here by the strong positive correlation between the tendency of the flame to be displaced and the measured amplitude of pressure pulsations. (author)

  9. Laser induced fluorescence measurements and modeling of nitric oxide in high-pressure premixed flames

    NASA Technical Reports Server (NTRS)

    Reisel, John R.; Laurendeau, Normand M.

    1994-01-01

    Laser-induced fluorescence (LIF) has been applied to the quantitative measurement of nitric oxide (NO) in premixed, laminar, high-pressure flames. Their chemistry was also studied using three current kinetics schemes to determine the predictive capabilities of each mechanism with respect to NO concentrations. The flames studied were low-temperature (1600 less than T less than 1850K) C2H6/O2/N2 and C2H6/O2/N2 flames, and high temperature (2100 less than T less than 2300K) C2H6/O2/N2 flames. Laser-saturated fluorescence (LSF) was initially used to measure the NO concentrations. However, while the excitation transition was well saturated at atmospheric pressure, the fluorescence behavior was basically linear with respect to laser power at pressures above 6 atm. Measurements and calculations demonstrated that the fluorescence quenching rate variation is negligible for LIF measurements of NO at a given pressure. Therefore, linear LIF was used to perform quantitative measurements of NO concentration in these high-pressure flames. The transportability of a calibration factor from one set of flame conditions to another also was investigated by considering changes in the absorption and quenching environment for different flame conditions. The feasibility of performing LIF measurements of (NO) in turbulent flames was studied; the single-shot detection limit was determined to be 2 ppm.

  10. Hydrodynamic theory of premixed flames: effects of stoichiometry, variable transport coefficients and arbitrary reaction orders

    NASA Astrophysics Data System (ADS)

    Matalon, M.; Cui, C.; Bechtold, J. K.

    2003-07-01

    Based on a hydrodynamic length, which is typically larger than the nominal flame thickness, a premixed flame can be viewed as a surface of density discontinuity, advected and distorted by the flow. The velocities and the pressure suffer abrupt changes across the flame front that consist of Rankine Hugoniot jump conditions, to leading order, with corrections of the order of the flame thickness that account for transverse fluxes and accumulation. To complete the formulation, expressions for the flame temperature and propagation speed, which vary along the flame as a result of local non-uniformities in the flow field and of flame front curvature, are derived. Unlike previous studies that assumed a mixture consisting of a single deficient reactant, the present study uses a two-reactant scheme and thus considers mixtures whose compositions vary from lean to rich conditions. Furthermore, non-unity and general reaction orders are considered in an attempt to mimic a wider range of reaction mechanisms and, to better represent actual experimental conditions, all transport coefficients are allowed to depend arbitrarily on temperature. The present model, expressed in a coordinate-free form, is valid for flames of arbitrary shape propagating in general fluid flows, either laminar or turbulent.

  11. Markstein Numbers of Negatively-Stretched Premixed Flames: Microgravity Measurements and Computations

    NASA Technical Reports Server (NTRS)

    Ibarreta, Alfonso F.; Driscoll, James F.; Feikema, Douglas A.; Salzman, Jack (Technical Monitor)

    2001-01-01

    The effect of flame stretch, composed of strain and curvature, plays a major role in the propagation of turbulent premixed flames. Although all forms of stretch (positive and negative) are present in turbulent conditions, little research has been focused on the stretch due to curvature. The present study quantifies the Markstein number (which characterizes the sensitivity of the flame propagation speed to the imposed stretch rate) for an inwardly-propagating flame (IPF). This flame is of interest because it is negatively stretched, and is subjected to curvature effects alone, without the competing effects of strain. In an extension of our previous work, microgravity experiments were run using a vortex-flame interaction to create a pocket of reactants surrounded by an IPF. Computations using the RUN-1DL code of Rogg were also performed in order to explain the measurements. It was found that the Markstein number of an inwardly-propagating flame, for both the microgravity experiment and the computations, is significantly larger than that of an outwardly-propagating flame. Further insight was gained by running the computations for the simplified (hypothetical) cases of one step chemistry, unity Lewis number, and negligible heat release. Results provide additional evidence that the Markstein numbers associated with strain and curvature have different values.

  12. Experimental and numerical study of premixed hydrogen/air flame propagating in a combustion chamber.

    PubMed

    Xiao, Huahua; Sun, Jinhua; Chen, Peng

    2014-03-15

    An experimental and numerical study of dynamics of premixed hydrogen/air flame in a closed explosion vessel is described. High-speed shlieren cinematography and pressure recording are used to elucidate the dynamics of the combustion process in the experiment. A dynamically thickened flame model associated with a detailed reaction mechanism is employed in the numerical simulation to examine the flame-flow interaction and effect of wall friction on the flame dynamics. The shlieren photographs show that the flame develops into a distorted tulip shape after a well-pronounced classical tulip front has been formed. The experimental results reveal that the distorted tulip flame disappears with the primary tulip cusp and the distortions merging into each other, and then a classical tulip is repeated. The combustion dynamics is reasonably reproduced in the numerical simulations, including the variations in flame shape and position, pressure build-up and periodically oscillating behavior. It is found that both the tulip and distorted tulip flames can be created in the simulation with free-slip boundary condition at the walls of the vessel and behave in a manner quite close to that in the experiments. This means that the wall friction could be unimportant for the tulip and distorted tulip formation although the boundary layer formed along the sidewalls has an influence to a certain extent on the flame behavior near the sidewalls. The distorted tulip flame is also observed to be produced in the absence of vortex flow in the numerical simulations. The TF model with a detailed chemical scheme is reliable for investigating the dynamics of distorted tulip flame propagation and its underlying mechanism. PMID:24486615

  13. Straining and wrinkling processes during turbulence-premixed flame interaction measured using temporally-resolved diagnostics

    SciTech Connect

    Steinberg, Adam M.; Driscoll, James F.

    2009-12-15

    The dynamical processes of flame surface straining and wrinkling that occur as turbulence interacts with a premixed flame were measured using cinema-stereoscopic PIV (CS-PIV) and orthogonal-plane cinema-stereoscopic PIV (OPCS-PIV). These diagnostics provided temporally resolved measurements of turbulence-flame interaction at frame rates of up to 3 kHz and spatial resolutions as small as 280{mu} m. Previous descriptions of flame straining and wrinkling have typically been derived based on a canonical interaction between a pair of counter-rotating vortices and a planar flame surface. However, it was found that this configuration did not properly represent real turbulence-flame interaction. Interactions resembling the canonical configuration were observed in less than 10% of the recorded frames. Instead, straining and wrinkling were generally caused more geometrically complex turbulence, consisting of large groups of structures that could be multiply curved and intertwined. The effect of the interaction was highly dependent on the interaction geometry. Furthermore, even when the turbulence did exist in the canonical geometry, the straining and wrinkling of the flame surface were not well characterized by the vortical structures. A new mechanistic description of the turbulence-flame interaction was therefore identified and confirmed by the measurements. In this description, flame surface straining is caused by coherent structures of fluid-dynamic strain-rate (strain-rate structures). The role of vortical structures is to curve existing flame surface, creating wrinkles. By simultaneously considering both forms of turbulent structure, turbulence-flame interactions in both the canonical configuration and more complex geometries could be understood. (author)

  14. Laser ablation plasma-assisted stabilization of premixed methane/air flame

    NASA Astrophysics Data System (ADS)

    Li, Xiaohui; Yu, Yang; Peng, Jiangbo; Yu, Xin; Fan, Rongwei; Sun, Rui; Chen, Deying

    2016-01-01

    Laser ablation plasma has been applied to assist stabilization of premixed methane/air flames with a flow speed up to 15.3 m/s. The ablation plasma was generated using the 50 Hz, 1064 nm output of a Nd:YAG laser onto a tantalum slab. With the ablation plasma, the stabilization equivalence ratio has been extended to the fuel-leaner end and the blow off limits have been enhanced by from 3.6- to 14.8-folds for flames which can stabilize without the plasma. The laser pulse energy required for flameholding was reduced to 10 mJ, a 64 % reduction compared with that of gas breakdown plasma, which will ease the demand for high-power lasers for high-frequency plasma generation. The temporal evolutions of the flame kernels following the ablation plasma were investigated using the OH* chemiluminescence imaging approach, and the flame propagation speed ( v f) was measured from the flame kernel evolutions. With the ablation plasma, the v f with flow speed of 4.7-9.0 m/s and equivalence ratio of 1.4 has been enhanced from 0.175 m/s of laminar premixed methane/air flame to 2.79-4.52 and 1.59-5.46 m/s, respectively, in the early and late time following the ablation plasma. The increase in the combustion radical concentrations by the ablation plasma was thought to be responsible for the v f enhancement and the resulted flame stabilization.

  15. Near field flow structure of isothermal swirling flows and reacting non-premixed swirling flames

    SciTech Connect

    Olivani, Andrea; Solero, Giulio; Cozzi, Fabio; Coghe, Aldo

    2007-04-15

    Two confined lean non-premixed swirl-stabilized flame typologies were investigated in order to achieve detailed information on the thermal and aerodynamic field in the close vicinity of the burner throat and provide correlation with the exhaust emissions. Previous finding indicated the generation of a partially premixed flame with radial fuel injection and a purely diffusive flame with co-axial injection in a swirling co-flow. In the present work, the experimental study is reported which has been conducted on a straight exit laboratory burner with no quarl cone, fuelled by natural gas and air, and fired vertically upwards with the flame stabilized at the end of two concentric pipes with the annulus supplying swirled air and the central pipe delivering the fuel. Two fuel injection typologies, co-axial and radial (i.e., transverse), leading to different mixing mechanisms, have been characterized through different techniques: particle image velocimetry (PIV) and laser Doppler velocimetry (LDV) for a comprehensive analysis of the velocity field, still photography for the detection of flame front and main visible features, and thermocouples for the temperature distribution. Isothermal flow conditions have been included in the experimental investigation to provide a basic picture of the flow field and to comprehend the modifications induced by the combustion process. The results indicated that, although the global mixing process and the main flame structure are governed by the swirl motion imparted to the air stream, the two different fuel injection methodologies play an important role on mixture formation and flame stabilization in the primary mixing zone. Particularly, it has been found that, in case of axial injection, the turbulent interaction between the central fuel jet and the backflow generated by the swirl can induce an intermittent fuel penetration in the recirculated hot products and the formation of a central sooting luminous plume, a phenomenon totally

  16. Effects of Radiative and Diffusive Transport Processes on Premixed Flames near Flammability Limits

    NASA Technical Reports Server (NTRS)

    Abbud-Madrid, Angel; Ronney, Paul D.

    1991-01-01

    A study of the mechanisms of flammability limits and the dynamics of flame extinguishment in premixed gas flames is described, a novel feature of which is the use of diluent gases having a wide range of radiative and diffusive transport properties. This feature enables an assessment of the importance of volumetric heat losses and Lewis number effects on these mechanisms. Additionally, effects of flame dynamics and flame front curvature are studied by employing spherically expanding flames obtained in a microgravity environment whereby natural convection is eliminated. New diagnostics include chamber pressure measurements and the first reported species concentration measurements in a microgravity combustion experiment. The limit mechanisms and extinguishment phenomena are found to be strongly influenced by the combined effects of radiant heat loss, Lewis number and flame curvature. Two new and as yet not well understood phenomena are reported: 'double flames' in rich H2-O2-CO2 mixtures and an 'inverse flammability region' in rich C3H8-O2-CO2 mixtures.

  17. An Experimental Study of the Structure of Turbulent Non-Premixed Jet Flames in Microgravity

    NASA Astrophysics Data System (ADS)

    Boxx, Isaac; Idicheria, Cherian; Clemens, Noel

    2000-11-01

    The aim of this work is to investigate the structure of transitional and turbulent non-premixed jet flames under microgravity conditions. The microgravity experiments are being conducted using a newly developed drop rig and the University of Texas 1.5 second drop tower. The rig itself measures 16”x33”x38” and contains a co-flowing round jet flame facility, flow control system, CCD camera, and data/image acquisition computer. These experiments are the first phase of a larger study being conducted at the NASA Glenn Research Center 2.2 second drop tower facility. The flames being studied include methane and propane round jet flames at jet exit Reynolds numbers as high as 10,000. The primary diagnostic technique employed is emission imaging of flame luminosity using a relatively high-speed (350 fps) CCD camera. The high-speed images are used to study flame height, flame tip dynamics and burnout characteristics. Results are compared to normal gravity experimental results obtained in the same apparatus.

  18. Local quenching phenomena of a lean premixed flat flame impinging with a pulsating air jet

    NASA Astrophysics Data System (ADS)

    Yahagi, Y.; Makino, I.

    2014-08-01

    Local quenching phenomena of a lean methane air premixed flat flame formed horizontally in a wall stagnating flow impinging with a pulsating air jet has been investigated experimentally. The burner system consists of 40mm inverted nozzle burner and a solid wall with 8mm diameter air jet placed in line vertically. The pulsating frequencies set up to 100Hz while the jet intensities generate up to 6 m/s by a loud speaker. Approximately '00mm disk shape flame front is curved by the pulsating air jet and the air jet impacting point is locally quenched. The fuel concentration of quenching start condition increases with increasing the intensity of air jet, because the increased jet intensity linked with the flame strain rate gain. For weak jet intensity range, the quenching hole becomes directly to develop the whole flame extinction. On the other hand, for moderate or strong jet condition, the flame can recover from the local quenching phenomena. In this condition, once the quenching hole creates, but the hole may close by the flame propagation or reigniting process. Then, the whole flame extinction limits are lower than no jet impacting condition depending on the circumstances.

  19. A numerical and experimental investigation of premixed methane-air flame transient response

    SciTech Connect

    Habib N. Najm; Phillip H. Paul; Omar M. Knio; Andrew McIlroy

    2000-01-06

    The authors report the results of a numerical and experimental investigation of the response of premixed methane-air flames to transient strain-rate disturbances induced by a two-dimensional counter-rotating vortex-pair. The numerical and experimental time histories of flow and flame evolution are matched over a 10 ms interaction time. Measurements and computations of CH and OH peak data evolution are reported, and found to indicate mis-prediction of the flame time scales in the numerical model. Qualitative transient features of OH at rich conditions are not predicted in the computations. On the other hand, evolution of computed and measured normalized HCO fractions are in agreement. The computed CH{sub 3}O response exhibits a strong transient driven by changes to internal flame structure, namely temperature profile steepening, induced by the flow field. Steady state experimental PLIF CH{sub 3}O data is reported, but experimental transient CH{sub 3}O data is not available. The present analysis indicates that the flame responds at time scales that are quite distinct from ``propagation'' time scale derived from flame thickness and burning speed. Evidently, these propagation time scales are not adequate for characterizing the transient flame response.

  20. Numerical simulations of turbulent premixed H2/O2/N2 flames with complex chemistry

    NASA Technical Reports Server (NTRS)

    Baum, M.; Poinsot, T. J.; Haworth, D. C.

    1992-01-01

    Premixed stoichiometric H2/O2/N2 flames propagating in two-dimensional turbulence were studied using direct numerical simulation (simulations in which all fluid and thermochemical scales are fully resolved) including realistic chemical kinetics and molecular transport. Results are compared with earlier zero-chemistry (flame sheet) and one-step chemistry simulations. Consistent with the simpler models, the turbulent flame with realistic chemistry aligns preferentially with extensive strain rates in the tangent plane and flame curvature probability density functions are close to symmetric with near-zero means. By contrast to simple-chemistry results with non-unity Lewis numbers (ratio of thermal to species diffusivity), local flame structure does not correlate with curvature but rather with tangential strain rate. Turbulent straining results in substantial thinning of the flame relative to the steady unstrained laminar case. Heat release and H2O2 contours remain thin and connected ('flamelet-like') while species including H-atom and OH are more diffuse. Peak OH concentration occurs well behind the peak heat-release zone. The feasibility of incorporating realistic chemistry into full turbulence simulations to address issues such as pollutant formation in hydrocarbon-air flames is suggested.

  1. Effects of Lewis number on turbulent scalar transport and its modelling in turbulent premixed flames

    SciTech Connect

    Chakraborty, Nilanjan; Cant, R.S.

    2009-07-15

    The behaviour of the turbulent scalar flux in premixed flames has been studied using Direct Numerical Simulation (DNS) with emphasis on the effects of Lewis number in the context of Reynolds-averaged closure modelling. A database was obtained from DNS of three-dimensional freely propagating statistically planar turbulent premixed flames with simplified chemistry and a range of global Lewis numbers from 0.34 to 1.2. Under the same initial conditions of turbulence, flames with low Lewis numbers are found to exhibit counter-gradient transport, whereas flames with higher Lewis numbers tend to exhibit gradient transport. The Reynolds-averaged transport equation for the turbulent scalar flux is analysed in detail and the performance of existing models for the unclosed terms is assessed with respect to corresponding quantities extracted from DNS data. Based on this assessment, existing models which are able to address the effects of non-unity Lewis number on turbulent scalar flux transport are identified, and new or modified models are suggested wherever necessary. In this way, a complete set of closure models for the scalar flux transport equation is prescribed for use in Reynolds-Averaged Navier-Stokes simulations. (author)

  2. OH-Planar Fluorescence Measurements of Pressurized, Hydrogen Premixed Flames in the SimVal Combustor

    SciTech Connect

    Strakey, P.A.; Woodruff, S.D.; Williams, T.C.; Schefer, R.W.

    2008-07-01

    Planar laser-induced fluorescence measurements of the hydroxyl radical in lean, premixed natural gas flames augmented with hydrogen are presented. The experiments were conducted in the Simulation Validation combustor at the National Energy Technology Laboratory at operating pressures from 1 to 8 atmospheres. The data, which were collected in a combustor with well-controlled boundary conditions, are intended to be used for validating computational fluid dynamics models under conditions directly relevant to land-based gas turbine engines. The images, which show significant effects of hydrogen on local flame quenching, are discussed in terms of a turbulent premixed combustion regime and nondimensional parameters such as Karlovitz number. Pressure was found to thin the OH region, but only had a secondary effect on overall flame shape compared with the effects of hydrogen addition, which was found to decrease local quenching and shorten the turbulent flame brush. A method to process the individual images based on local gradients of fluorescence intensity is proposed, and results are presented. Finally, the results of several large eddy simulations are presented and compared with the experimental data in an effort to understand the issues related to model validation, especially for simulations that do not include OH as an intermediate species.

  3. Geometrical properties of turbulent premixed flames and other corrugated interfaces

    NASA Astrophysics Data System (ADS)

    Thiesset, F.; Maurice, G.; Halter, F.; Mazellier, N.; Chauveau, C.; Gökalp, I.

    2016-01-01

    This study focuses on the geometrical properties of turbulent flame fronts and other interfaces. Toward that end, we use an original tool based on proper orthogonal decomposition (POD), which is applied to the interface spatial coordinates. The focus is mainly on the degree of roughness of the flame front, which is quantified through the scale dependence of its coverage arclength. POD is first validated by comparing with the caliper technique. Fractal characteristics are extracted in an unambiguous fashion using a parametric expression which appears to be impressively well suited for representing Richardson plots. Then it is shown that, for the range of Reynolds numbers investigated here, the scale-by-scale contribution to the arclength does not comply with scale similarity, irrespectively of the type of similarity which is invoked. The finite ratios between large and small scales, referred to as finite Reynolds number effects, are likely to explain this observation. In this context, the Reynolds number that ought to be achieved for a proper inertial range to be discernible, and for scale similarity to be likely to apply, is calculated. Fractal characteristics of flame folding are compared to available predictions. It is confirmed that the inner cutoff satisfactorily correlates with the Kolmogorov scale while the outer cutoff appears to be proportional to the integral length scale. However, the scaling for the fractal dimension is much less obvious. It is argued that much higher Reynolds numbers have to be reached for drawing firm statements about the evolution (or constancy) of the fractal dimension with respect to flame and flow parameters. Finally, a heuristic phenomenology of corrugated interfaces is highlighted. The degree of generality of the latter phenomenology is confirmed by comparing the folding of different interfaces including a turbulent-nonturbulent interface, a liquid jet destabilized by a surrounding air jet, a cavitating flow, and an isoscalar

  4. Geometrical properties of turbulent premixed flames and other corrugated interfaces.

    PubMed

    Thiesset, F; Maurice, G; Halter, F; Mazellier, N; Chauveau, C; Gökalp, I

    2016-01-01

    This study focuses on the geometrical properties of turbulent flame fronts and other interfaces. Toward that end, we use an original tool based on proper orthogonal decomposition (POD), which is applied to the interface spatial coordinates. The focus is mainly on the degree of roughness of the flame front, which is quantified through the scale dependence of its coverage arclength. POD is first validated by comparing with the caliper technique. Fractal characteristics are extracted in an unambiguous fashion using a parametric expression which appears to be impressively well suited for representing Richardson plots. Then it is shown that, for the range of Reynolds numbers investigated here, the scale-by-scale contribution to the arclength does not comply with scale similarity, irrespectively of the type of similarity which is invoked. The finite ratios between large and small scales, referred to as finite Reynolds number effects, are likely to explain this observation. In this context, the Reynolds number that ought to be achieved for a proper inertial range to be discernible, and for scale similarity to be likely to apply, is calculated. Fractal characteristics of flame folding are compared to available predictions. It is confirmed that the inner cutoff satisfactorily correlates with the Kolmogorov scale while the outer cutoff appears to be proportional to the integral length scale. However, the scaling for the fractal dimension is much less obvious. It is argued that much higher Reynolds numbers have to be reached for drawing firm statements about the evolution (or constancy) of the fractal dimension with respect to flame and flow parameters. Finally, a heuristic phenomenology of corrugated interfaces is highlighted. The degree of generality of the latter phenomenology is confirmed by comparing the folding of different interfaces including a turbulent-nonturbulent interface, a liquid jet destabilized by a surrounding air jet, a cavitating flow, and an isoscalar

  5. Quantifying real-gas effects on a laminar n-dodecane - air premixed flame

    NASA Astrophysics Data System (ADS)

    Gopal, Abishek; Yellapantula, Shashank; Larsson, Johan

    2015-11-01

    With the increasing demand for higher efficiencies in aircraft gas-turbine engines, there has been a progressive march towards high pressure-ratio cycles. Under these conditions, the aviation fuel, Jet A, is injected into the combustor at supercritical pressures. In this work, we study and quantify the effects of transcriticality on a 1D freely propagating laminar n-dodecane - air premixed flame. The impact of the constitutive state relations arising from the Ideal Gas equation of state(EOS) and Peng-Robinson EOS on flame structure and propagation is presented. The effects of real-gas models of transport properties, such as viscosity on laminar flame speed, are also presented.

  6. Non-premixed flame-turbulence interaction in compressible turbulent flow

    SciTech Connect

    Livescu, D.; Madnia, C. K.

    2002-01-01

    Nonpremixed turbulent reacting flows are intrinsically difficult to model due to the strong coupling between turbulent motions and reaction. The large amount of heat released by a typical hydrocarbon flame leads to significant modifications of the thermodynamic variables and the molecular transport coefficients and thus alters the fluid dynamics. Additionally, in nonpremixed combustion, the flame has a complex spatial structure. Localized expansions and contractions occur, enhancing the dilatational motions. Therefore, the compressibility of the flow and the heat release are intimately related. However, fundamental studies of the role of compressibility on the scalar mixing and reaction are scarce. In this paper they present results concerning the fundamental aspects of the interaction between non-premixed flame and compressible turbulence.

  7. A detailed kinetic modeling study of aromatics formation in laminar premixed acetylene and ethylene flames

    SciTech Connect

    Wang, H.; Frenklach, M.

    1997-07-01

    A computational study was performed for the formation and growth of polycyclic aromatic hydrocarbons (PAHs) in laminar premixed acetylene and ethylene flames. A new detailed reaction mechanism describing fuel pyrolysis and oxidation, benzene formation, and PAH mass growth and oxidation is presented and critically tested. It is shown that the reaction model predicts reasonably well the concentration profiles of major and intermediate species and aromatic molecules in a number of acetylene and ethylene flames reported in the literature. It is demonstrated that reactions of n-C{sub 4}H{sub x} + C{sub 2}H{sub 2} leading to the formation of one-ring aromatics are as important as the propargyl recombination, and hence must be included in kinetic modeling of PAH formation in hydrocarbon flames. It is further demonstrated that the mass growth of PAHs can be accounted for by the previously proposed H-abstraction-C{sub 2}H{sub 2}-addiction mechanism.

  8. Potential-flow models for channelled two-dimensional premixed flames around near-circular obstacles

    NASA Astrophysics Data System (ADS)

    Joulin, G.; Denet, B.; El-Rabii, H.

    2010-01-01

    The dynamics of two-dimensional thin premixed flames is addressed in the framework of mathematical models where the flow field on either side of the front is piecewise incompressible and vorticity free. Flames confined in channels with asymptotically straight impenetrable walls are considered. Besides a few free propagations along straight channels, attention is focused on flames propagating against high-speed flows and positioned near a round central obstacle or near two symmetric bumps protruding inward. Combining conformal maps and Green’s functions, a regularized generalization of Frankel’s integro-differential equation for the instantaneous front shape in each configuration is derived and solved numerically. This produces a variety of real looking phenomena: steady fronts (symmetric or not), noise-induced subwrinkles, flashback events, and breathing fronts in pulsating flows. Perspectives and open mathematical and physical problems are finally evoked.

  9. The influence of pressure on the control of premixed turbulent flames using an electric field

    SciTech Connect

    Sakhrieh, A.; Dinkelacker, F.; Leipertz, A.; Lins, G.; Hammer, T.; Branston, D.W.

    2005-11-01

    Previous investigations of the effects of electric fields on flames have shown the potential for stabilizing flames and reducing emissions with comparatively little effort, but were restricted to atmospheric pressure. In the present work the influence of the electric field on premixed turbulent jet flames at increased pressure is investigated. Besides the question of whether field effects persist at elevated pressure, it is of interest to find physically based scaling laws. The current work describes experiments with premixed turbulent seven-hole Bunsen-jet flames for pressures between 1 and 10 bar, where the exit velocity was held constant, and where electric fields of varied strength and direction were applied to the flame. Concentrations of CO, NO, and NO{sub 2} were measured in the exhaust gas section. Experiments show that the electric field influence is clearly visible for increased pressures, without any indication that 10 bar should be an upper limit. CO emissions could be reduced by about 95%, irrespective of pressure. The decrease of CO was accompanied by an increase of NO{sub x} by about 25%. Both of these effects can be understood qualitatively within the framework of a one-dimensional model. For reduced voltages up to 3.5 kV/bar the model correctly describes the current-voltage characteristics and leads to the conclusion that high pressure should favor rather than hamper electric field effects on flames. The electric power required for a CO reduction of 95% amounted to 0.1% of the thermal power. The improvement of the lean blowoff limit upon application of an electric field observed so far ranges from 1 to 3% and increases with pressure.

  10. Analyzing and Tracking Burning Structures in Lean Premixed Hydrogen Flames

    SciTech Connect

    Bremer, Peer-Timo; Weber, Gunther; Pascucci, Valerio; Day, Marc; Bell, John

    2009-06-01

    This paper presents topology-based methods to robustly extract, analyze, and track features defined as subsets of isosurfaces. First, we demonstrate how features identified by thresholding isosurfaces can be defined in terms of the Morse complex. Second, we present a specialized hierarchy that encodes the feature segmentation independent of the threshold while still providing a flexible multi-resolution representation. Third, for a given parameter selection we create detailed tracking graphs representing the complete evolution of all features in a combustion simulation over several hundred time steps. Finally, we discuss a user interface that correlates the tracking information with interactive rendering of the segmented isosurfaces enabling an in-depth analysis of the temporal behavior. We demonstrate our approach by analyzing three numerical simulations of lean hydrogen flames subject to different levels of turbulence. Due to their unstable nature, lean flames burn in cells separated by locally extinguished regions. The number, area, and evolution over time of these cells provide important insights into the impact of turbulence on the combustion process. Utilizing the hierarchy we can perform an extensive parameter study without re-processing the data for each set of parameters. The resulting statistics enable scientist to select appropriate parameters and provide insight into the sensitivity of the results wrt. to the choice of parameters. Our method allows for the first time to quantitatively correlate the turbulence of the burning process with the distribution of burning regions, properly segmented and selected. In particular, our analysis shows that counter-intuitively stronger turbulence leads to larger cell structures, which burn more intensely than expected. This behavior suggests that flames could be stabilized under much leaner conditions than previously anticipated.

  11. Effects of Buoyancy on Lean Premixed V-Flames Part I: Laminar and Turblent Flame Structure

    NASA Technical Reports Server (NTRS)

    Cheng, Robert K.; Bedat, Benoit; Kostiuk, Larry W.

    1998-01-01

    Laser schlieren and planar laser-induced fluorescence techniques have been used to investigate laminar and turbulent v-flames in +g, -g, and micro g under flow conditions that span the regimes of momentum domination (Ri < 0. 1) and buoyancy domination (Ri > 0.1). Overall flame features shown by schlieren indicate that buoyancy dominates the entire flow field for conditions close to Ri = 1. With decreasing Ri, buoyancy effects are observed only in the far-field regions. Analyses of the mean flame angles demonstrate that laminar and turbulent flames do not have similar responses to buoyancy. Difference in the laminar +g and -g flame angles decrease with Ri (i.e., increasing Re) and converge to the microgravity flame angle at the momentum limit (Ri - 0). This is consistent with the notion that the effects of buoyancy diminish with increasing flow momentum. The +g and -g turbulent flame angles, however, do not converge at Ri = 0. As shown by OH-PLIF images, the inconsistency in +g and -g turbulent flame angles is associated with the differences in flame wrinkles. Turbulent flame wrinkles evolve more slowly in +g than in -g. The difference in flame wrinkle structures, however, cannot be explained in terms of buoyancy effects on flame instability mechanisms. It seems to be associated with the field effects of buoyancy that stretches the turbulent flame brushes in +g and compresses the flame brush in -g. Flame wrinkling offers a mechanism through which the flame responds to the field effects of buoyancy despite increasing flow momentum. These observations point to the need to include both upstream and downstream contributions in theoretical analysis of flame turbulence interactions.

  12. Geometrical properties of turbulent premixed flames and other corrugated interfaces.

    PubMed

    Thiesset, F; Maurice, G; Halter, F; Mazellier, N; Chauveau, C; Gökalp, I

    2016-01-01

    This study focuses on the geometrical properties of turbulent flame fronts and other interfaces. Toward that end, we use an original tool based on proper orthogonal decomposition (POD), which is applied to the interface spatial coordinates. The focus is mainly on the degree of roughness of the flame front, which is quantified through the scale dependence of its coverage arclength. POD is first validated by comparing with the caliper technique. Fractal characteristics are extracted in an unambiguous fashion using a parametric expression which appears to be impressively well suited for representing Richardson plots. Then it is shown that, for the range of Reynolds numbers investigated here, the scale-by-scale contribution to the arclength does not comply with scale similarity, irrespectively of the type of similarity which is invoked. The finite ratios between large and small scales, referred to as finite Reynolds number effects, are likely to explain this observation. In this context, the Reynolds number that ought to be achieved for a proper inertial range to be discernible, and for scale similarity to be likely to apply, is calculated. Fractal characteristics of flame folding are compared to available predictions. It is confirmed that the inner cutoff satisfactorily correlates with the Kolmogorov scale while the outer cutoff appears to be proportional to the integral length scale. However, the scaling for the fractal dimension is much less obvious. It is argued that much higher Reynolds numbers have to be reached for drawing firm statements about the evolution (or constancy) of the fractal dimension with respect to flame and flow parameters. Finally, a heuristic phenomenology of corrugated interfaces is highlighted. The degree of generality of the latter phenomenology is confirmed by comparing the folding of different interfaces including a turbulent-nonturbulent interface, a liquid jet destabilized by a surrounding air jet, a cavitating flow, and an isoscalar

  13. Direct numerical simulations of turbulent non-premixed methane-air flames modeled with reduced kinetics

    NASA Technical Reports Server (NTRS)

    Card, J. M.; Chen, J. H.; Day, M.; Mahalingam, S.

    1994-01-01

    Turbulent non-premixed stoichiometric methane-air flames modeled with reduced kinetics have been studied using the direct numerical simulation approach. The simulations include realistic chemical kinetics, and the molecular transport is modeled with constant Lewis numbers for individual species. The effect of turbulence on the internal flame structure and extinction characteristics of methane-air flames is evaluated. Consistent with earlier DNS with simple one-step chemistry, the flame is wrinkled and in some regions extinguished by the turbulence, while the turbulence is weakened in the vicinity of the flame due to a combination of dilatation and an increase in kinematic viscosity. Unlike previous results, reignition is observed in the present simulations. Lewis number effects are important in determining the local stoichiometry of the flame. The results presented in this work are preliminary but demonstrate the feasibility of incorporating reduced kinetics for the oxidation of methane with direct numerical simulations of homogeneous turbulence to evaluate the limitations of various levels of reduction in the kinetics and to address the formation of thermal and prompt NO(x).

  14. Soot volume fraction in a piloted turbulent jet non-premixed flame of natural gas

    SciTech Connect

    Qamar, N.H.; Alwahabi, Z.T.; King, K.D.; Chan, Q.N.; Nathan, G.J.; Roekaerts, D.

    2009-07-15

    Planar laser-induced incandescence (LII) has been used to measure soot volume fraction in a well-characterised, piloted, turbulent non-premixed flame known as the ''Delft Flame III''. Simulated Dutch natural gas was used as the fuel to produce a flame closely matching those in which a wide range of previous investigations, both experimental and modelling, have been performed. The LII method was calibrated using a Santoro-style burner with ethylene as the fuel. Instantaneous and time-averaged data of the axial and radial soot volume fraction distributions of the flame are presented here along with the Probability Density Functions (PDFs) and intermittency. The PDFs were found to be well-characterised by a single exponential distribution function. The distribution of soot was found to be highly intermittent, with intermittency typically exceeding 97%, which increases measurement uncertainty. The instantaneous values of volume fraction are everywhere less than the values in strained laminar flames. This is consistent with the soot being found locally in strained flame sheets that are convected and distorted by the flow. (author)

  15. Quasi-steady stages in the process of premixed flame acceleration in narrow channels

    NASA Astrophysics Data System (ADS)

    Valiev, D. M.; Bychkov, V.; Akkerman, V.; Eriksson, L.-E.; Law, C. K.

    2013-09-01

    The present paper addresses the phenomenon of spontaneous acceleration of a premixed flame front propagating in micro-channels, with subsequent deflagration-to-detonation transition. It has recently been shown experimentally [M. Wu, M. Burke, S. Son, and R. Yetter, Proc. Combust. Inst. 31, 2429 (2007)], 10.1016/j.proci.2006.08.098, computationally [D. Valiev, V. Bychkov, V. Akkerman, and L.-E. Eriksson, Phys. Rev. E 80, 036317 (2009)], 10.1103/PhysRevE.80.036317, and analytically [V. Bychkov, V. Akkerman, D. Valiev, and C. K. Law, Phys. Rev. E 81, 026309 (2010)], 10.1103/PhysRevE.81.026309 that the flame acceleration undergoes different stages, from an initial exponential regime to quasi-steady fast deflagration with saturated velocity. The present work focuses on the final saturation stages in the process of flame acceleration, when the flame propagates with supersonic velocity with respect to the channel walls. It is shown that an intermediate stage may occur during acceleration with quasi-steady velocity, noticeably below the Chapman-Jouguet deflagration speed. The intermediate stage is followed by additional flame acceleration and subsequent saturation to the Chapman-Jouguet deflagration regime. We elucidate the intermediate stage by the joint effect of gas pre-compression ahead of the flame front and the hydraulic resistance. The additional acceleration is related to viscous heating at the channel walls, being of key importance at the final stages. The possibility of explosion triggering is also demonstrated.

  16. Radical Concentrations and Prompt NO Formation in Hydrocarbon-Air Premixed Flames

    NASA Astrophysics Data System (ADS)

    Matusi, Yasuji; Yuuki, Akimasa

    1985-05-01

    Hydroxyl radical concentrations in laminar, premixed CH4-air flat-flames were measured by a conventional absorption method in the flame temperature range T{=}2200-1700 K. The OH mole fractions in the reaction zone POH were found to be insensitive to the flame temperature and the maximum POH to be about 6× 10-3 at T{=}2000 K in a stoichiometric flame. The rate constant for the prompt NO formation, CH+N2→HCN+N\\dashrightarrow2NO (4), is modified as k4{=}1.2× 1012\\exp (-13600/RT) by the relation between the amount of prompt NO and the saturation ion current Is. It is also shown from the measurements of NOx, unburnt hydrocarbons H.C., and Is, that the chemical kinetics are not significantly influenced by the flame temperature, and NO emission is reduced by reactions among NO, H.C., and N-containing intermediate species in low-temperature flames, even in stoichiometric and fuel-lean mixtures.

  17. Response dynamics of bluff-body stabilized conical premixed turbulent flames with spatial mixture gradients

    SciTech Connect

    Chaudhuri, Swetaprovo; Cetegen, Baki M.

    2009-03-15

    Response of bluff-body stabilized conical turbulent premixed flames was experimentally studied for a range of excitation frequencies (10-400 Hz), mean flow velocities (5, 10 and 15 m/s) and three different spatial mixture distributions (uniform, inner and outer enrichment). Upstream excitation was provided by a loudspeaker producing velocity oscillation amplitudes of about 8% of the mean flow velocity. Flame response was detected by a photomultiplier observing the CH{sup *} emission from the flame. The studied turbulent flames exhibited transfer function characteristics of a low-pass filter with a cutoff Strouhal number between 0.08 and 0.12. The amplification factors at low frequencies ranged from 2 to 20 and generally increased for mean flow velocities from 5 to 15 m/s. The highest levels of amplification were found for the outer mixture enrichment followed in decreasing order by uniform and inner mixture gradient cases. The high levels of flame response for the outer enrichment case were attributed to the enhanced flame-vortex interaction in outer jet shear layer. At high excitation levels (u{sup '}/U{sub m}{approx}0.3) for U{sub m}=5 m/ s where non-linear flame response is expected, the flame exhibited a reduced amplitude response in the frequency range between 40 and 100 Hz for the uniform and outer equivalence ratio gradient cases and no discernible effect for the inner equivalence ratio gradient. In all cases, transfer function phase was found to vary linearly with excitation frequency. Finally, a relationship between the amplitude characteristics of the bluff-body wake transfer function and flame blowoff equivalence ratio was presented. (author)

  18. Large eddy simulation of soot formation in a turbulent non-premixed jet flame

    SciTech Connect

    El-Asrag, Hossam; Menon, Suresh

    2009-02-15

    A recently developed subgrid model for soot dynamics [H. El-Asrag, T. Lu, C.K. Law, S. Menon, Combust. Flame 150 (2007) 108-126] is used to study the soot formation in a non-premixed turbulent flame. The model allows coupling between reaction, diffusion and soot (including soot diffusion and thermophoretic forces) processes in the subgrid domain without requiring ad hoc filtering or model parameter adjustments. The combined model includes the entire process, from the initial phase, when the soot nucleus diameter is much smaller than the mean free path, to the final phase, after coagulation and aggregation, where it can be considered in the continuum regime. A relatively detailed but reduced kinetics for ethylene-air is used to simulate an experimentally studied non-premixed ethylene/air jet diffusion flame. Acetylene is used as a soot precursor species. The soot volume fraction order of magnitude, the location of its maxima, and the soot particle size distribution are all captured reasonably. Along the centerline, an initial region dominated by nucleation and surface growth is established followed by an oxidation region. The diffusion effect is found to be most important in the nucleation regime, while the thermophoretic forces become more influential downstream of the potential core in the oxidation zone. The particle size distribution shows a log-normal distribution in the nucleation region, and a more Gaussian like distribution further downstream. Limitations of the current approach and possible solution strategies are also discussed. (author)

  19. Large eddy simulation of a lean premixed swirl flame in complex geometry - comparison of two turbulent combustion models

    NASA Astrophysics Data System (ADS)

    Wang, P.; Fröhlich, J.; Maas, U.

    Lean premixed combustion is employed to reduce emission, but can exhibit undesired effects such as lean blow-off and thermo-acoustic resonance. To cope with these, burners with strong swirl are utilized for flame stabilization. In the resulting complex flow system, flow instabilities are observed in both experiments and simulations. To date, large eddy simulation (LES) is becoming a widely used approach for understanding the properties of turbulent flow phenomena. However, LES of lean premixed combustion still constitutes an open challenge. Many turbulent combustion modeling methods have been developed for LES of such flows [1, 2]. Two types of them are the thickened flame (TF) model [3] and the flame surface density (FSD) model [4]. However, none of these models is ideal and suitable for all kinds of flame configurations. A detailed comparison was made between the TF and FSD by Lin et al. [5] for freely propagating premixed flames in homogeneous isotropic decaying turbulent fields, and qualitative agreement between them was found. In the present work, the performances of the two cited turbulent combustion models, TF and FSD, in simulating the lean premixed swirl flames in an industrial gas trubine model combustor is compared against the well-documented experiment data obtained by Meier et al. [6].

  20. Tulip flames: changes in shape of premixed flames propagating in closed tubes

    NASA Astrophysics Data System (ADS)

    Dunn-Rankin, D.; Sawyer, R. F.

    The experimental results that are the subject of this communication provide high-speed schlieren images of the closed-tube flame shape that has come to be known as the tulip flame. The schlieren images, along with in-chamber pressure records, help demonstrate the effects of chamber length, equivalence ratio, and igniter geometry on formation of the tulip flame. The pressure/time records show distinct features which correlate with flame shape changes during the transition to tulip. The measurements indicate that the basic tulip flame formation is a robust phenomenon that depends on little except the overall geometry of the combustion vessel.

  1. Relationships for maximum flame surface density and brush thickness through conditional analysis in turbulent premixed combustion

    NASA Astrophysics Data System (ADS)

    Huh, Kang Y.; Kwon, Jaesung; Lee, Dongkyu

    2013-07-01

    A new conditional averaging method is introduced in terms of the reaction progress variable, c, and its derivatives of successively higher orders, Σ _f^' (or -∂c/∂n) and ∂2c/∂n2, in high Damköhler number (Da) turbulent premixed combustion. c is continuous and differentiable in space so that conditional averages may be defined for flamelets of finite thicknesses as well as for infinitesimally thin flamelets. A coupled set of transport equations are derived with corresponding conditional coefficient terms for mean reaction progress variable, bar c, and flame surface density (FSD), Σf. Statistics for all component terms are consistent with previous results and show the same qualitative trends irrespective of compressibility by the new averaging practice. It is shown that the maximum FSD, Σmax, occurs at the location where the relationship, nabla ^2 bar c + < {nabla \\cdot {n}} rangle _f Σ _f = 0, holds in a flame brush. An analytical expression is derived for Σmax under the assumption of constant tangential strain rate and linear variation of mean curvature and mean displacement speed, ⟨Sd⟩f, in the bar c space. Σmax becomes equal to one fourth ⟨|∇.n|⟩f or half the mean absolute curvature for fully turbulent flames with the magnitude of ⟨n⟩f close to zero. Once the turbulent burning velocity, ST, is determined by asymptotic behavior at the leading edge, the brush thickness, ℓF, may be obtained from local and integral relationships for the product, ℓFΣmax, in a steadily propagating one-dimensional flame. The newly proposed relationships reproduce proper trends of variation for ST, Σmax, and ℓF against measurement data in literature. They are validated to show good agreement with direct numerical simulation (DNS) results of the Lewis number equal to unity for freely propagating incompressible and stagnating compressible turbulent premixed flames.

  2. Study and modeling of finite rate chemistry effects in turbulent non-premixed flames

    NASA Technical Reports Server (NTRS)

    Vervisch, Luc

    1993-01-01

    The development of numerical models that reflect some of the most important features of turbulent reacting flows requires information about the behavior of key quantities in well defined combustion regimes. In turbulent flames, the coupling between turbulent and chemical processes is so strong that it is extremely difficult to isolate the role played by one individual physical phenomenon. Direct numerical simulation (hereafter DNS) allows us to study in detail the turbulence-chemistry interaction in some restricted but completely defined situations. Globally, non-premixed flames are controlled by two limiting regimes: the fast chemistry case, where the turbulent flame can be pictured as a random distribution of local chemical equilibrium problems; and the slow chemistry case, where the chemistry integrates in time the turbulent fluctuations. The Damkoehler number, ratio of a mechanical time scale to chemical time scale, is used to distinguish between these regimes. Today most of the industrial computer codes are able to perform predictions in the hypothesis of local equilibrium chemistry using a presumed shape for the probability density function (pdt) of the conserved scalar. However, the finite rate chemistry situation is of great interest because industrial burners usually generate regimes in which, at some points, the flame is undergoing local extinction or at least non-equilibrium situations. Moreover, this variety of situations strongly influences the production of pollutants. To quantify finite rate chemistry effect, the interaction between a non-premixed flame and a free decaying turbulence is studied using DNS. The attention is focused on the dynamic of extinction, and an attempt is made to quantify the effect of the reaction on the small scale mixing process. The unequal diffusivity effect is also addressed. Finally, a simple turbulent combustion model based on the DNS observations and tractable in real flow configurations is proposed.

  3. Effects of differential diffusion on the flame structure of oxygen enhanced turbulent non-premixed jet flames

    NASA Astrophysics Data System (ADS)

    Dietzsch, Felix; Gauding, Michael; Hasse, Christian

    2014-11-01

    By means of Direct Numerical Simulation we have investigated the influence of differential diffusion for non-premixed oxygen-enhanced turbulent flames. Oxygen-enhanced conversion usually yields higher amounts of H2 as compared to conventional air combustion. It is well known that H2 as a very diffusive species leads to differential diffusion effects. In addition to the diffusive transport mixing processes are also often controlled by turbulent transport. Previous investigations of a turbulent CH4/H2 oxygen-enhanced jet flame have shown that in mixture fraction space it is important to distinguish between regions of equal diffusivities and detailed transport. These findings are of particular interest when performing Large-Eddy simulations applying a flamelet approach. Using this approach a LES study was performed of the aforementioned flame considering differential diffusion. Therefore, flamelet equations including differential diffusion via non-unity constant Lewis numbers were solved. However, this study showed that keeping the non-unity Lewis numbers constant, is not sufficient to capture the diffusion phenomena in this particular flame. Direct Numerical Simulations have been conducted in order to investigate how Lewis numbers are affected in mixture fraction space. Computer resources for this project have been provided by the Gauss Centre for Supercomputing/Leibniz Supercomputing Centre under Grant: pr83xa.

  4. Combustion oscillation monitoring using flame ionization in a turbulent premixed combustor

    SciTech Connect

    Chorpening, B.T.; Thornton, J.D.; Huckaby, E.D.; Benson, K.J.

    2007-04-01

    To achieve very low NOx emission levels, lean-premixed gas turbine combustors have been commercially implemented that operate near the fuel-lean flame extinction limit. Near the lean limit, however, flashback, lean blow off, and combustion dynamics have appeared as problems during operation. To help address these operational problems, a combustion control and diagnostics sensor (CCADS) for gas turbine combustors is being developed. CCADS uses the electrical properties of the flame to detect key events and monitor critical operating parameters within the combustor. Previous development efforts have shown the capability of CCADS to monitor flashback and equivalence ratio. Recent work has focused on detecting and measuring combustion instabilities. A highly instrumented atmospheric combustor has been used to measure the pressure oscillations in the combustor, the OH emission, and the flame ion field at the premix injector outlet and along the walls of the combustor. This instrumentation allows examination of the downstream extent of the combustion field using both the OH emission and the corresponding electron and ion distribution near the walls of the combustor. In most cases, the strongest pressure oscillation dominates the frequency behavior of the OH emission and the flame ion signals. Using this highly instrumented combustor, tests were run over a matrix of equivalence ratios from 0.6 to 0.8, with an inlet reference velocity of 25 m/s 82 ft/ s . The acoustics of the fuel system for the combustor were tuned using an active-passive technique with an adjustable quarter-wave resonator. Although several statistics were investigated for correlation with the dynamic pressure in the combustor, the best correlation was found with the standard deviation of the guard current. The data show a monotonic relationship between the standard deviation of the guard current (the current through the flame at the premix injector outlet) and the standard deviation of the chamber

  5. The effects of ferrocene addition on soot particle inception and growth in premixed ethylene flames

    SciTech Connect

    Ritrievi, K.E.; Longwell, J.P.; Sarofim, A.F.

    1987-10-01

    The effects of the addition of dicyclopentadienyl iron, ferrocene, on soot particle inception and growth were studied in atmospheric pressure, premixed ethylene flames with C/O = 0.71-0.83 at 0.015-0.46% ferrocene by weight of the fuel. The rate of surface growth of soot in undoped and doped flames was measured using laser light scattering and light extinction techniques to determine the particle size and number density as a function of residence time in the flame. The final soot yields in the ferrocene doped flames were enhanced by factors of 13.5-1.2 over the range of flame C/O ratios studied. This enhancement decreased with increasing C/O ratio for the same concentration of iron in the flames. The spatial distribution of the elements iron and carbon in the particles was determined with Auger spectroscopy. The iron was found to be concentrated in the cores of the particles. The results of a steady-state one-dimensional nucleation model which indicated that the iron oxide particles would nucleate well in advance of the soot inception time were consistent with this elemental stratification and the observation of the onset of carbon deposition in doped flames at earlier residence times than in undoped flames of the same C/O ratio. The iron oxide particle sizes and number densities predicted from the model indicated that these particles were both numerous and small enough to be seed particles on which carbon deposition could take place. The importance of the activity of the surfaces of the solid in determining the rate of surface growth of soot was investigated.

  6. Control of oscillations and NOx concentrations in ducted premixed flames by spray injection of water

    SciTech Connect

    Sivasegaram, S.; Tsai, R.F.; Whitelaw, J.H.

    1995-12-31

    The antinodal rms pressure fluctuations of a ducted premixed flame has been reduced from 9 to 1.75 kPa by pulsed injection of water with heat removal of less than 3% of the total heat release of 150 kW. A corresponding benefit was the reduction in NO{sub x} emissions from 65 to 30 ppm. Several control strategies were considered and active control based on the oscillation of injection at the same phase as that of the oscillations was found to provide the best combination of attenuation and NO{sub x} reduction.

  7. Analysis of the electric currents in 1D premixed flames under applied voltages

    NASA Astrophysics Data System (ADS)

    Han, Jie; Belhi, Memdouh; Bisetti, Fabrizio; Casey, Tiernan; Im, Hong G.; Chen, Jyh-Yuan

    2015-11-01

    Studying electric currents in flames has practical aspects such as the determination of the ionic structure of a flame, the analysis of the flame behavior under an electric field and the use of flame electric properties for combustion diagnostics. This study proposes a simplified model to compute the electric currents in lean-to-stoichiometric 1D premixed flames under applied voltages. The Navier-Stokes equations coupled with transport equations for neutral and charged species along with a Poisson equation for the electric potential are solved. The model reproduces qualitatively the voltage-current characteristic found experimentally. The sensitivity of the electric currents to the applied voltage, equivalence ratio, and pressure is studied and the key parameters affecting the saturation current are determined. Results show that the saturation current is controlled by the amount of charged species created by the chemi-ionization reaction. We found that the recombination rate of electrons with cations and transport coefficients of charged species are the most important parameters affecting the voltage at witch saturation occurs. Analytical formulas for the voltage-current characteristic and the potential of saturation are developed and used to explain the obtained results.

  8. Simultaneous krypton PLIF, LII and PIV measurements in a sooting non-premixed jet flame

    NASA Astrophysics Data System (ADS)

    Buxton, Oliver; Burns, Ross; Clemens, Noel

    2012-11-01

    Simultaneous krypton planar laser induced fluorescence (PLIF), laser induced incandescence (LII) and stereoscopic PIV measurements are made in a sooting jet flame for the first time. Krypton is seeded into the jet stream to provide a conserved scalar marker from which mixture fraction can be inferred. 2% krypton is seeded into a non-premixed ethylene/nitrogen jet flame with a cold jet Reynolds number based on bulk velocity of 5100. An electronic transition is accessed through a two photon excitation using an incident 214.7 nm light sheet, producing fluorescence at 760 nm. This fluorescence is spectrally isolated from the flame's bulk luminescence and PAH fluorescence. The fluorescence signal can then be converted to mixture fraction by measuring the relative krypton quenching rates of the various species present in the flame core and making use of a flamelet-based chemical state relationship. This technique is used simultaneously with LII, which will provide the soot volume fraction, and stereoscopic PIV which will provide all three velocity components in a plane. It will thus be possible to observe the influence of the velocity field on the formation and transport of soot, and the evolution of mixture fraction, and its effect on soot formation, within the sooting jet flame.

  9. Effect of a uniform electric field on soot in laminar premixed ethylene/air flames

    SciTech Connect

    Wang, Y.; Yao, Q.; Nathan, G.J.; Alwahabi, Z.T.; King, K.D.; Ho, K.

    2010-07-15

    The effect of a nominally uniform electric field on the initially uniform distribution of soot has been assessed for laminar premixed ethylene/air flames from a McKenna burner. An electrophoretic influence on charged soot particles was measured through changes to the deposition rate of soot on the McKenna plug, using laser extinction (LE). Soot volume fraction was measured in situ using laser-induced incandescence (LII). Particle size and morphologies were assessed through ex situ transmission electron microscopy (TEM) using thermophoretic sampling particle diagnostics (TSPD). The results show that the majority of these soot particles are positively charged. The presence of a negatively charged plug was found to decrease the particle residence times in the flame and to influence the formation and oxidation progress. A positively charged plug has the opposite effect. The effect on soot volume fraction, particles size and morphology with electric field strength is also reported. Flame stability was also found to be affected by the presence of the electric field, with the balance of the electrophoretic force and drag force controlling the transition to unstable flame flicker. The presence of charged species generated by the flame was found to reduce the dielectric field strength to one seventh that of air. (author)

  10. Measurements of fuel mixture fraction oscillations of a turbulent jet non-premixed flame

    SciTech Connect

    Kanga, D.M.; Fernandez, V.; Culick, F.E.C.; Ratner, A.

    2009-01-15

    This work describes new type of combustion instability for which the 3-way coupling between mixing, flame heat release, and acoustics is modified by local buoyancy effects. Measurements of fuel mixture fraction are made for a non-premixed jet flame in a combustion chamber to assess the dynamics of mixing under imposed acoustic oscillations (22-55 Hz). Infrared laser absorption and phase resolved acetone-planar laser induced fluorescence are used to measure the fuel mixture fraction and then the degree of fuel/air mixing is calculated by determining the unmixedness. Results show acoustic excitation causes oscillations in the degree of fuel/air mixing at the driving frequency, which results in oscillatory flame behavior. This oscillatory flame behavior couples to the buoyancy and this in turn affects the mixing. Results also show that the mixing becomes less effective when the excitation frequency is increased or when the flame is present, compared to the non-reacting case. This work describes a key coupling mechanism that occurs when buoyancy is a significant factor in the flow field. (author)

  11. Experimental and modeling investigation of aromatic and polycyclic aromatic hydrocarbon formation in a premixed ethylene flame

    SciTech Connect

    Castaldi, M.J.; Marinov, N.M.; Melius, C.F.

    1996-02-01

    Experimental and detailed chemical kinetic modeling has been performed to investigate aromatic and polyaromatic hydrocarbon formation pathways in a rich, sooting, ethylene-oxygen-argon premixed flame. An atmospheric pressure, laminar flat flame operated at an equivalence ratio of 2.5 was used to acquire experimental data for model validation. Gas composition analysis was conducted by an on-line gas chromatograph/mass spectrometer (GC/MS) technique. Measurements were made in the flame and post-flame zone for a number of low molecular weight species, aliphatics, aromatics and polycyclic aromatic hydrocarbons (PAHs) ranging from two to five-aromatic fused rings. The modeling results show the key reaction sequences leading to aromatic and polycyclic aromatic hydrocarbon growth involve the combination of resonantly stabilized radicals. In particular, propargyl and 1-methylallenyl combination reactions lead to benzene and methyl substituted benzene formation, while polycyclic aromatics are formed from cyclopentadienyl radicals and fused rings that have a shared C{sub 5} side structure. Naphthalene production through the reaction step of cyclopentadienyl self-combination and phenanthrene formation from indenyl and cyclopentadienyl combination were shown to be important in the flame modeling study. The removal of phenyl by O{sub 2} leading to cyclopentadienyl formation is expected to play a pivotal role in the PAH or soot precursor growth process under fuel-rich oxidation conditions.

  12. An experimental and kinetic investigation of premixed furan/oxygen/argon flames

    PubMed Central

    Tian, Zhenyu; Yuan, Tao; Fournet, Rene; Glaude, Pierre-Alexandre; Sirjean, Baptiste; Battin-Leclerc, Frédérique; Zhang, Kuiwen; Qi, Fei

    2013-01-01

    The detailed chemical structures of three low-pressure (35 Torr) premixed laminar furan/oxygen/argon flames with equivalence ratios of 1.4, 1.8 and 2.2 have been investigated by using tunable synchrotron vacuum ultraviolet (VUV) photoionization and molecular-beam mass spectrometry. About 40 combustion species including hydrocarbons and oxygenated intermediates have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of the flame species including reactants, intermediates and products have been determined by scanning burner position with some selected photon energies near ionization thresholds. Flame temperatures have been measured by a Pt-6%Rh/Pt-30%Rh thermocouple. A new mechanism involving 206 species and 1368 reactions has been proposed whose predictions are in reasonable agreement with measured species profiles for the three investigated flames. Rate-of-production and sensitivity analyses have been performed to track the key reaction paths governing furan consumption for different equivalence ratios. Both experimental and modeling results indicate that few aromatics could be formed in these flames. Furthermore, the current model has been validated against previous pyrolysis results of the literature obtained behind shock waves and the agreement is reasonable as well. PMID:23814311

  13. Structure of the Soot Growth Region of Laminar Premixed Methane/Oxygen Flames. Appendix I

    NASA Technical Reports Server (NTRS)

    Xu, F.; Faeth, G. M.; Urban, D. L. (Technical Monitor); Yuan, Z.-G. (Technical Monitor)

    2001-01-01

    The structure of the soot growth region of laminar premixed methane/oxygen flames (fuel-equivalence ratios of 1.60-2.77) was studied both experimentally and computationally. Measurements were carried out in flames stabilized on a flat flame burner operated at standard temperature and pressure, and included velocities by laser velocimetry, soot volume fractions by laser extinction, soot temperatures by multiline emission, gas temperatures (where soot was absent) by corrected fine-wire thermocouples, major gas species concentrations by sampling and gas chromatography, and hydrogen atom concentrations by the Li/LiOH technique in conjunction with atomic absorption to find the proportion of free lithium in the flames. The measured concentrations of major gas species were in reasonably good agreement with predictions based on the detailed mechanisms of Leung and Lindstedt, and Frenklach and coworkers. The measurements also confirmed predictions of both these mechanisms that H-atom concentrations are in local thermodynamic equilibrium throughout the soot growth region even through the concentrations of major gas species are not. Thus, present findings support recent evaluations of the hydrogen-abstraction/carbon-addition (HACA) soot growth mechanism in similar flames, where the approximation that H-atom concentrations were in local thermodynamic equilibrium was adopted, based on predictions using the two mechanisms, due to the absence of direct H-atom concentration measurements.

  14. Structure of Soot Growth Region of Laminar Premixed Methane/Oxygen Flames. Appendix B

    NASA Technical Reports Server (NTRS)

    Xu, F.; Faeth, G. M.; Urban, D. L. (Technical Monitor); Yuan, Z.-G. (Technical Monitor)

    2000-01-01

    The structure of the soot growth region of laminar premixed methane/oxygen flames (fuel-equivalence ratios of 1.60 - 2.77) was studied both experimentally and computationally. Measurements were carried out in flames stabilized on a flat flame burner operated at standard temperature and pressure, and included velocities by laser velocimetry, soot volume fractions by laser extinction, soot temperatures by multiline emission, gas temperatures (where soot was absent) by corrected fine-wire thermocouples, major gas species concentrations by sampling and gas chromatography, and hydrogen atom concentrations by the Li/LiOH technique in conjunction with atomic absorption to find the proportion of free lithium in the flames. The measured concentrations of major gas species were in reasonably good agreement with predictions based on the detailed mechanisms of Leung and Lindstedt, and Frenklach and coworkers. The measurements also confirmed predictions of both these mechanisms that H-atom concentrations are in local thermodynamic equilibrium throughout the soot growth region even through the concentrations of major gas species are not. Thus, present findings support recent evaluations of the hydrogen-abstraction/carbon-addition (HACA) soot growth mechanism in similar flames, where the approximation that H-atom concentrations were in local thermodynamic equilibrium was adopted, based on predictions using the two mechanisms, due to the absence of direct H-atom concentration measurements.

  15. Structure of the Soot Growth Region of Laminar Premixed Methane/Oxygen Flames. Appendix G

    NASA Technical Reports Server (NTRS)

    Xu, F.; Faeth, G. M.; Yuan, Z.-G. (Technical Monitor); Urban, D. L. (Technical Monitor); Yuan, Z.-G. (Technical Monitor)

    2000-01-01

    The structure of the soot growth region of laminar premixed methane/oxygen flames (fuel-equivalence ratios of 1.60-2.77) was studied both experimentally and computationally. Measurements were carried out in flames stabilized on a flat flame burner operated at standard temperature and pressure, and included velocities by laser velocimetry, soot volume fractions by laser extinction, soot temperatures by multiline emission, gas temperatures (where soot was absent) by corrected fine-wire thermocouples, major gas species concentrations by sampling and gas chromatography, and hydrogen atom concentrations by the Li/LiOH technique in conjunction with atomic absorption to find the proportion of free lithium in the flames. The measured concentrations of major gas species were in reasonably good agreement with predictions based on the detailed mechanisms of Leung and Lindstedt, and Frenklach and coworkers. The measurements also confirmed predictions of both these mechanisms that H-atom concentrations are in local thermodynamic equilibrium throughout the soot growth region even through the concentrations of major gas species are not. Thus, present findings support recent evaluations of the hydrogen-abstraction/carbon-addition (HACA) soot growth mechanism in similar flames, where the approximation that H-atom concentrations were in local thermodynamic equilibrium was adopted, based on predictions using the two mechanisms, due to the absence of direct H-atom concentration measurements.

  16. Aromatic and polycyclic aromatic hydrocarbon formation in a laminar premixed n-butane flame

    SciTech Connect

    Marinov, N.M.; Pitz, W.J.; Westbrook, C.K.; Vincitore, A.M.; Castaldi, M.J.; Senkan, S.M.; Melius, C.F.

    1998-07-01

    Experimental and detailed chemical kinetic modeling work has been performed to investigate aromatic and polycyclic aromatic hydrocarbon (PAH) formation pathways in a premixed, rich, sooting, n-butane-oxygen-argon burner stabilized flame. An atmospheric pressure, laminar flat flame operated at an equivalence ratio of 2.6 was used to acquire experimental data for model validation. Gas composition analysis was conducted by an on-line gas chromatograph/mass spectrometer technique. Measurements were made in the main reaction and post-reaction zones for a number of low molecular weight species, aliphatics, aromatics, and polycyclic aromatic hydrocarbons (PAHs) ranging from two to five-fused aromatic rings. Reaction flux and sensitivity analysis were used to help identify the important reaction sequences leading to aromatic and PAH growth and destruction in the n-butane flame. Reaction flux analysis showed the propargyl recombination reaction was the dominant pathway to benzene formation. The consumption of propargyl by H atoms was shown to limit propargyl, benzene, and naphthalene formation in flames as exhibited by the large negative sensitivity coefficients. Naphthalene and phenanthrene production was shown to be plausibly formed through reactions involving resonantly stabilized cyclopentadienyl and indenyl radicals. Many of the low molecular weight aliphatics, combustion by-products, aromatics, branched aromatics, and PAHs were fairly well simulated by the model. Additional work is required to understand the formation mechanisms of phenyl acetylene, pyrene, and fluoranthene in the n-butane flame. 73 refs.

  17. VUV Photoionization Study of the Allyl Radical from Premixed Gasoline/Oxygen Flame

    NASA Astrophysics Data System (ADS)

    Yang, Rui; Yang, Bin; Huang, Chao-qun; Wei, Li-xia; Wang, Jing; Shan, Xiao-bin; Sheng, Liu-si; Zhang, Yun-wu; Qi, Fei; Yao, Chun-de; Li, Qi; Ji, Qing

    2006-02-01

    The allyl radical has been observed in a low-pressure premixed gasoline/oxygen/argon flame by using tunable vacuum ultraviolet photoionization mass spectrometry. The ionization potential of the allyl radical is derived to be (8.13 ± 0.02) eV from photoionization efficiency curve. In addition, a high level ab initio Gaussian-3 (G3) method was used to calculate the energies of the radical and its cation. The calculated adiabatic ionization potential is 8.18 eV, which is in excellent agreement with the experimental value. The result is helpful for identifying the allyl radical formed from other flames and for understanding the mechanism of soot formation.

  18. LDA measurements in the premixed V flame stabilized in the wake of a flat plate boundary layer

    SciTech Connect

    Trevino, C. ); Donnerhack, S. ); Peters, N. )

    1991-06-01

    This paper presents laser-doppler measurements and particle track photographs of V-shaped flame. The flame is stabilized behind a splitter plate in a two-dimensional premixed gas flow. In order to stabilize the flame, the splitter plate must be heated, indicating the importance of the thermal interaction between the flame and the plate. Based on theoretical concepts of the viscous flow at the trailing edge of a plate, an order of magnitude of the thermal penetration length is performed. This is compared with the preheat zone thickness.

  19. A direct numerical simulation study of vorticity transformation in weakly turbulent premixed flames

    NASA Astrophysics Data System (ADS)

    Lipatnikov, A. N.; Nishiki, S.; Hasegawa, T.

    2014-10-01

    Database obtained earlier in 3D Direct Numerical Simulations (DNS) of statistically stationary, 1D, planar turbulent flames characterized by three different density ratios σ is processed in order to investigate vorticity transformation in premixed combustion under conditions of moderately weak turbulence (rms turbulent velocity and laminar flame speed are roughly equal to one another). In cases H and M characterized by σ = 7.53 and 5.0, respectively, anisotropic generation of vorticity within the flame brush is reported. In order to study physical mechanisms that control this phenomenon, various terms in vorticity and enstrophy balance equations are analyzed, with both mean terms and terms conditioned on a particular value c of the combustion progress variable being addressed. Results indicate an important role played by baroclinic torque and dilatation in transformation of average vorticity and enstrophy within both flamelets and flame brush. Besides these widely recognized physical mechanisms, two other effects are documented. First, viscous stresses redistribute enstrophy within flamelets, but play a minor role in the balance of the mean enstrophy overline{Ω } within turbulent flame brush. Second, negative correlation overline{mathbf {u}^' } \\cdot nabla Ω ^' }} between fluctuations in velocity u and enstrophy gradient contributes substantially to an increase in the mean overline{Ω } within turbulent flame brush. This negative correlation is mainly controlled by the positive correlation between fluctuations in the enstrophy and dilatation and, therefore, dilatation fluctuations substantially reduce the damping effect of the mean dilatation on the vorticity and enstrophy fields. In case L characterized by σ = 2.5, these effects are weakly pronounced and overline{Ω } is reduced mainly due to viscosity. Under conditions of the present DNS, vortex stretching plays a minor role in the balance of vorticity and enstrophy within turbulent flame brush in all three

  20. Flame front surface characteristics in turbulent premixed propane/air combustion

    SciTech Connect

    Guelder, O.L.; Smallwood, G.J.; Wong, R.; Snelling, D.R.; Smith, R.; Deschamps, B.M.; Sautet, J.C.

    2000-03-01

    The characteristics of the flame front surfaces in turbulent premixed propane/air flames were investigated. Flame front images were obtained using laser-induced fluorescence (LIF) of OH and Mie scattering on two Bunsen-type burners of 11.2-mm and 22.4-mm diameters. Nondimensional turbulence intensity, u{prime}/S{sub L}, was varied from 0.9 to 15, and the Reynolds number, based on the integral length scale, varied from 40 to 467. Approximately 100 images were recorded for each experimental condition. Fractal parameters (fractal dimension, inner and outer cutoffs) and corresponding standard deviations were determined by analysis of the flame front images using the caliper technique. The fractal dimensions derived from OH and Mie scattering images are almost identical. However, inner and outer cutoffs from OH images are consistently higher than those obtained from Mie scattering. The self-similar region of the flame front wrinkling is about a decade for all flames studied. In the nondimensional turbulence intensity range from 1 to 15, it was found that the mean fractal dimension is about 2.2 and it does not show any dependence on turbulence intensity. This contradicts the findings of the previous studies that showed that the fractal dimension asymptotically reaches to 2.35--2.37 when the nondimensional turbulence intensity u{prime}/S{sub L} exceeds 3. It is shown that the reason for this discrepancy is the image analysis method used in the previous studies. Examples are given to show the inadequacy of the circle method used in previous studies for extraction of fractal parameters from flame front images. The fractal parameters obtained so far, in this and previous studies, are not capable of correctly predicting the turbulent burning velocity using the available fractal area closure model.

  1. Modeling ignition and chemical structure of partially premixed turbulent flames using tabulated chemistry

    SciTech Connect

    Michel, Jean-Baptiste; Colin, Olivier; Veynante, Denis

    2008-01-15

    Correctly reproducing the autoignition and the chemical composition of partially premixed turbulent flames is a challenge for numerical simulations of industrial applications such as diesel engines. A new model DF-PCM (diffusion flame presumed conditional moment) is proposed based on a coupling between the FPI (flame prolongation of ILDM) tabulation method and the PCM (presumed conditional moment) approach. Because the flamelets used to build the table are laminar diffusion flames, DF-PCM cannot be used for industrial applications like Diesel engines due to excessive CPU requirements. Therefore two new models called AI-PCM (autoignition presumed conditional moment) and ADF-PCM (approximated diffusion flames presumed conditional moment) are developed to approximate it. These models differ from DF-PCM because the flamelet libraries used for the table rely on PSR calculations. Comparisons between DF-PCM, AI-PCM, and ADF-PCM are performed for two fuels, n-heptane, representative of diesel fuels, and methane, which does not exhibit a ''cool flame'' ignition regime. These comparisons show that laminar diffusion flames can be approximated by flamelets based on PSR calculations in terms of autoignition delays and steady state profiles of the progress variable. Moreover, the evolution of the mean progress variable of DF-PCM can be correctly estimated by the approximated models. However, as discussed in this paper, errors are larger for CO and CO{sub 2} mass fractions evolutions. Finally, an improvement to ADF-PCM, taking into account ignition delays, is proposed to better reproduce the ignition of very rich mixtures. (author)

  2. Relevance of the Bray number in the small-scale modeling of turbulent premixed flames

    SciTech Connect

    Mura, Arnaud; Champion, Michel

    2009-03-15

    The present study is devoted to the analysis of the influence of expansion phenomena on turbulent small scales in premixed reactive flows. It is shown that, under certain conditions, the expansion that takes place across wrinkled laminar flamelet can be sufficient to control the fluctuating velocity gradients and associated dissipation rate functions. These conditions are fixed by the respective values of a set of nondimensional parameters, namely the turbulence Reynolds number Re{sub T}, the Bray number, and the ratio between integral length scale of turbulence and thermal flame front thickness. A new criterion is introduced that makes it possible to delineate the influence of expansion phenomena on small-scale turbulent premixed reactive flows. The relevance of this criterion is analyzed in the light of experimental results represented in the classical diagram of combustion regime. The present analysis confirms that special care is required to represent and include the influence of expansion phenomena when using either RANS or LES closures to model turbulent premixed combustion. (author)

  3. Computational study of lean premixed turbulent flames using RANSPDF and LESPDF methods

    NASA Astrophysics Data System (ADS)

    Rowinski, David H.; Pope, Stephen B.

    2013-08-01

    A computational study is performed on a series of four piloted, lean, premixed turbulent jet flames. These flames use the Sydney Piloted Premixed Jet Burner (PPJB), and with jet velocities of 50, 100, 150 and 200 m/s are denoted PM150, PM1100, PM1150 and PM1200, respectively. Calculations are performed using the RANSPDF and LESPDF methodologies, with different treatments of molecular diffusion, with detailed chemistry and flamelet-based chemistry modelling, and using different imposed boundary conditions. The sensitivities of the calculations to these different aspects of the modelling are compared and discussed. Comparisons are made to experimental data and to previously-performed calculations. It is found that, given suitable boundary conditions and treatment of molecular diffusion, excellent agreement between the calculations and experimental measurements of the mean and variance fields can be achieved for PM150 and PM1100. The application of a recently developed implementation of molecular diffusion results in a large improvement in the computed variance fields in the LESPDF calculations. The inclusion of differential diffusion in the LESPDF calculations provides insight on the behaviour in the near-field region of the jet, but its effects are found to be confined to this region and to the species CO, OH and H2. A major discrepancy observed in many previous calculations of these flames is an overprediction of reaction progress in PM1150 and PM1200, and this discrepancy is also observed in the LESPDF calculations; however, a parametric study of the LESPDF mixing model reveals that, with a sufficiently large mixing frequency, calculations of these two flames are capable of yielding improved reaction progress in good qualitative agreement with the mean and RMS scalar measurements up to an x/D of 30. Lastly, the merits of each computational methodology are discussed in light of their computational costs.

  4. Studies in premixed combustion

    SciTech Connect

    Sivashinsky, G.I.

    1992-01-01

    This report discusses the following topics on premixed combustion: theory of turbulent flame propagation; pattern formation in premixed flames and related problems; and pattern formation in extended systems. (LSP)

  5. Effects of CO addition on the characteristics of laminar premixed CH{sub 4}/air opposed-jet flames

    SciTech Connect

    Wu, C.-Y.; Chao, Y.-C.; Chen, C.-P.; Ho, C.-T.; Cheng, T.S.

    2009-02-15

    The effects of CO addition on the characteristics of premixed CH{sub 4}/air opposed-jet flames are investigated experimentally and numerically. Experimental measurements and numerical simulations of the flame front position, temperature, and velocity are performed in stoichiometric CH{sub 4}/CO/air opposed-jet flames with various CO contents in the fuel. Thermocouple is used for the determination of flame temperature, velocity measurement is made using particle image velocimetry (PIV), and the flame front position is measured by direct photograph as well as with laser-induced predissociative fluorescence (LIPF) of OH imaging techniques. The laminar burning velocity is calculated using the PREMIX code of Chemkin collection 3.5. The flame structures of the premixed stoichiometric CH{sub 4}/CO/air opposed-jet flames are simulated using the OPPDIF package with GRI-Mech 3.0 chemical kinetic mechanisms and detailed transport properties. The measured flame front position, temperature, and velocity of the stoichiometric CH{sub 4}/CO/air flames are closely predicted by the numerical calculations. Detailed analysis of the calculated chemical kinetic structures reveals that as the CO content in the fuel is increased from 0% to 80%, CO oxidation (R99) increases significantly and contributes to a significant level of heat-release rate. It is also shown that the laminar burning velocity reaches a maximum value (57.5 cm/s) at the condition of 80% of CO in the fuel. Based on the results of sensitivity analysis, the chemistry of CO consumption shifts to the dry oxidation kinetics when CO content is further increased over 80%. Comparison between the results of computed laminar burning velocity, flame temperature, CO consumption rate, and sensitivity analysis reveals that the effect of CO addition on the laminar burning velocity of the stoichiometric CH{sub 4}/CO/air flames is due mostly to the transition of the dominant chemical kinetic steps. (author)

  6. Examination of ionic wind and cathode sheath effects in a E-field premixed flame with ion density measurements

    NASA Astrophysics Data System (ADS)

    Jacobs, Stewart V.; Xu, Kunning G.

    2016-04-01

    The effect of the ionic wind on a premixed methane-air flame under a DC electric field is studied via mapping of the ion density with Langmuir probes. Ion densities were observed to increase near the burner with increasing electrode voltage up to 6 kV. Past this electrode supply voltage, ion densities ceased increasing and began to decline in some locations within the premixed flame. The increased ion density is caused by an increase in ionic wind force and cathode sheath thickness. The plateau in density is due to the cathode sheath fully encompassing the flame front which is the ion source, thereby collecting all ions in the flame. The spatial density data support the ionic wind hypothesis and provide further explanation of its limits based on the plasma sheath.

  7. Chemical kinetic considerations for postflame synthesis of carbon nanotubes in premixed flames using a support catalyst

    SciTech Connect

    Gopinath, Prarthana; Gore, Jay

    2007-11-15

    Multiwalled carbon nanotubes (MWCNTs) on a grid supported cobalt nanocatalyst were grown, by exposing it to combustion gases from ethylene/air rich premixed flames. Ten equivalence ratios ({phi}) were investigated, as follows: 1.37, 1.44, 1.47, 1.50, 1.55, 1.57, 1.62, 1.75, 1.82, and 1.91. MWCNT growth could be observed for the range of equivalence ratios between 1.45 and 1.75, with the best yield restricted to the range 1.5-1.6. A one-dimensional premixed flame code with a postflame heat loss model, including detailed chemistry, was used to estimate the gas phase chemical composition that favors MWCNT growth. The results of the calculations show that the mixture, including the water gas shift reaction, is not even in partial chemical equilibrium. Therefore, past discussions of compositional parameters that relate to optimum carbon nanotube (CNT) growth are revised to include chemical kinetic effects. Specifically, rapid departures of the water gas shift reaction from partial equilibrium and changes in mole fraction ratios of unburned C{sub 2} hydrocarbons to hydrogen correlate well with experimentally observed CNT yields. (author)

  8. A priori direct numerical simulation assessment of algebraic flame surface density models for turbulent premixed flames in the context of large eddy simulation

    NASA Astrophysics Data System (ADS)

    Chakraborty, Nilanjan; Klein, Markus

    2008-08-01

    Flame surface density (FSD) based reaction rate closure is one of the most important approaches in turbulent premixed flame modeling. The algebraic models for FSD based on power laws often require information about the fractal dimension D and the inner cut-off scale ηi. In the present study, two three-dimensional direct numerical simulation (DNS) databases for freely propagating statistically planar turbulent premixed flames are analyzed among which the flame in one case belongs to the corrugated flamelet (CF) regime, whereas the other falls well within the thin reaction zone (TRZ) regime. It is found that D for the flame in the TRZ regime is greater than the value obtained for the flame in the CF regime. For the flame within the TRZ regime, the fractal dimension is found to be 7/3, which is the same as D for a material surface in a turbulent environment. For the flame in the CF regime, ηi is found to scale with the Gibson scale, whereas ηi is found to scale with the Kolmogorov length scale for the flame in the TRZ regime. Based on these observations a new algebraic model for FSD is proposed, where D and ηi are expressed as functions of Karlovitz number. The performances of the new and existing algebraic models for FSD are compared with the corresponding values obtained from DNS databases.

  9. Turbulence measurements and observations of turbulent premixed flames at elevated pressures up to 3.0 MPa

    SciTech Connect

    Kobayashi, Hideaki; Maruta, Kaoru; Niioka, Takashi; Nakashima, Teppei; Tamura, Takashi

    1997-01-01

    In order to explore the characteristics of turbulence and turbulent premixed flames in a high-pressure environment, a nozzle-type burner with a turbulence generator was installed in a high-pressure chamber. Turbulence measurements and combustion experiments were conducted with the chamber pressure up to 3.0 MPa. Methane-air mixtures were used for the combustion experiments and confirmed that the turbulent premixed flames were successfully stabilized. Flame observations were made using instantaneous Schlieren photographs and high-speed laser tomography. Turbulence measurements were conducted using a hot-wire anemometer installed in the high-pressure chamber. It was found that the scales of turbulence generated by perforated plates at elevated pressure are smaller than those at atmospheric pressure. From flame observations, the following features of the flames at elevated pressure were found: (1) wrinkles structures of the flames become very fine and complex, and the cusps become sharp as pressure rises; (2) the flamelet breaks at many points of the flames and the scales of broken flamelets become small; (3) small-scale parts of the flame front convex to the unburned mixture frequently occur and move quickly to the unburned side. The effects of ambient pressure on turbulence characteristics and possible mechanisms which produce the wrinkled structure of the fine scales and generate flame front disturbances in the high-pressure environment are discussed.

  10. Flamelet/flow interaction in premixed turbulent flames: simultaneous measurements of gas velocity and flamelet position

    SciTech Connect

    Miles, P.C.; Gouldin, F.C.

    1996-12-01

    An experimental technique for obtaining simultaneous measurements of fluid velocity and flamelet position in premixed flames is described and applied in a turbulent V-flame. The flamelet position information is used to calculate conditional velocity statistics, conditional on both zone (reactants or products) as well as conditional on distance from the flamelet. The conditional zone statistics demonstrate that increases (or decreases) in turbulence across the flame are dependent on axial position and location within the flame brush. The product- zone conditional covariance, coupled with the measured conditional mean velocity profiles, indicate that turbulence generation by shear may be a significant contribution to product zone turbulence levels. Velocity statistics conditional on distance from the flamelet demonstrate a considerable interaction between the flamelet and velocity field. Man and rms velocities vary significantly with proximity to the flamelet, such that differences in velocities which which occur just across the flamelet surface. The change in rms velocities just across the flamelet is found to be anisotropic, with the largest increase (smallest decrease) occurring in the axial velocity component. Rms velocities conditional on flamelet position further support the hypothesis that increased product gas velocity fluctuations may have a significant component associated with turbulence generation by mean shear.

  11. A comparative study of TiO2 nanoparticles synthesized in premixed and diffusion flames

    NASA Astrophysics Data System (ADS)

    Ma, Hsiao-Kang; Yang, Hsiung-An

    2010-12-01

    Previous studies have been shown that synthesis of titania (TiO2) crystalline phase purity could be effectively controlled by the oxygen concentration through titanium tetra-isopropoxide (TTIP) via premixed flame from a Bunsen burner. In this study, a modified Hencken burner was used to synthesize smaller TiO2 nanoparticles via short diffusion flames. The frequency of collisions among particles would decrease and reduce TiO2 nanoparticle size in a short diffusion flame height. The crystalline structure of the synthesized nanoparticles was characterized by X-ray diffraction (XRD), transmission electron microscope (TEM), Barrett-Joyner-Halenda (BJH) and Brunauer-Emmett-Teller (BET) measurements. The characteristic properties of TiO2 nanoparticles synthesized from a modified Hencken burner were compared with the results from a Bunsen burner and commercial TiO2 (Degussa P25). The results showed that the average particle size of 6.63 nm from BET method was produced by a modified Hencken burner which was smaller than the TiO2 in a Bunsen burner and commercial TiO2. Moreover, the rutile content of TiO2 nanoparticles increased as the particle collecting height increased. Also, the size of TiO2 nanoparticles was highly dependent on the TTIP loading and the collecting height in the flame.

  12. Measurements of premixed-flame turbulence generation and modification in a Taylor-Couette burner

    SciTech Connect

    Arjomand-Kermani, Amir M.; Aldredge, Ralph C.

    2007-10-15

    Turbulent, premixed lean methane-air flames were studied experimentally in a Taylor-Couette burner, extending the previous work of non-reacting turbulent-flow measurements. A laser-Doppler velocimetry system is employed to measure velocity fluctuations in the circumferential direction at the center of the annulus where mean velocities are nearly zero. Turbulence parameters such as the intensities, approximated integral and micro-time and length scales and one-dimensional frequency spectra are obtained for the flow-field ahead and behind the flame front. The frequency spectra exhibit a -5/3 slope reaffirming isotropic characteristics. It is found that there is an increase in intensity, turbulence Reynolds number and energy across a broad range of frequencies behind the flame along with a shift toward larger scales. However, there appears to be a decrease in amplification of the intensities and turbulence Reynolds number with increasing pre-ignition turbulence in the burner (generated by counter-rotation of the cylinder walls). Results suggest that the presence of flame-generated turbulence in the TC burner is sensitive to both pre-ignition turbulence and equivalence ratio. (author)

  13. LIF measurements of turbulent premixed flames in a high pressure environment

    SciTech Connect

    Kobayashi, Hideaki; Oyachi, Yasuo; Maruta, Kaoru

    1999-07-01

    The effects of pressure on OH-LIF characteristics of laminar and turbulent premixed flames were investigated. OH-LIF experiments were performed for methane-air mixtures using burner flames stabilized in high-pressure chambers. An OPO tunable laser pumped by a Nd-YAG laser were used and A{sup 2}{Sigma}{sup +}-X{sup 2} II (0,0) and (1,0) band of OH radical were measured. For laminar flames, OH-LIF excitation spectrum was measured by scanning the laser wavelength at pressures up to 1.0 MPa. The overlap-integral profiles between Gaussian profiles of the laser and Voigt profiles of the absorption line were calculated, and the effects of pressure and laser linewidth on FWHM and intensities of the LIF excitation spectrum were compared with experimental data. Results show that the effects of pressure on the FWHM and peak intensity of overlap integral profiles agree qualitatively with those on the measured LIF excitation spectrum, indicating that the decrease in LIF intensity of the flame at high-pressure is dominated by the broadening of the absorption line shapes. The LIF intensity decreases with increasing linewidth of the laser. A narrow-band laser is effective in order to obtain higher LIF intensity at ordinary pressure but the linewidth of the laser has no significant effect at high pressures.

  14. The effect of nitrogen on biogas flame propagation characteristic in premix combustion

    NASA Astrophysics Data System (ADS)

    Anggono, Willyanto; Suprianto, Fandi D.; Hartanto, Tan Ivan; Purnomo, Kenny; Wijaya, Tubagus P.

    2016-03-01

    Biogas is one of alternative energy and categorized as renewable energy. The main sources of biogas come from animal waste, garbage, and household waste that are organic waste. Primarily, over 50% of this energy contains methane (CH4). The other substances or inhibitors are nitrogen and carbon dioxide. Previously, carbon dioxide effect on biogas combustion is already experimented. The result shows that carbon dioxide reduces the flame propagation speed of biogas combustion. Then, nitrogen as an inhibitor obviously also brings some effects to the biogas combustion, flame propagation speed, and flame characteristics. Spark ignited cylinder is used for the premixed biogas combustion research. An acrylic glass is used as the material of this transparent cylinder chamber. The cylinder is filled with methane (CH4), oxygen (O2), and nitrogen (N2) with particular percentage. In this experiment, the nitrogen composition are set to 0%, 5%, 10%, 20%, 30%, 40%, and 50%. The result shows that the flame propagation speed is reduced in regard to the increased level of nitrogen. It can also be implied that nitrogen can decrease the biogas combustion rate.

  15. Probe measurements and numerical model predictions of evolving size distributions in premixed flames

    SciTech Connect

    De Filippo, A.; Sgro, L.A.; Lanzuolo, G.; D'Alessio, A.

    2009-09-15

    Particle size distributions (PSDs), measured with a dilution probe and a Differential Mobility Analyzer (DMA), and numerical predictions of these PSDs, based on a model that includes only coagulation or alternatively inception and coagulation, are compared to investigate particle growth processes and possible sampling artifacts in the post-flame region of a C/O = 0.65 premixed laminar ethylene-air flame. Inputs to the numerical model are the PSD measured early in the flame (the initial condition for the aerosol population) and the temperature profile measured along the flame's axial centerline. The measured PSDs are initially unimodal, with a modal mobility diameter of 2.2 nm, and become bimodal later in the post-flame region. The smaller mode is best predicted with a size-dependent coagulation model, which allows some fraction of the smallest particles to escape collisions without resulting in coalescence or coagulation through the size-dependent coagulation efficiency ({gamma}{sub SD}). Instead, when {gamma} = 1 and the coagulation rate is equal to the collision rate for all particles regardless of their size, the coagulation model significantly under predicts the number concentration of both modes and over predicts the size of the largest particles in the distribution compared to the measured size distributions at various heights above the burner. The coagulation ({gamma}{sub SD}) model alone is unable to reproduce well the larger particle mode (mode II). Combining persistent nucleation with size-dependent coagulation brings the predicted PSDs to within experimental error of the measurements, which seems to suggest that surface growth processes are relatively insignificant in these flames. Shifting measured PSDs a few mm closer to the burner surface, generally adopted to correct for probe perturbations, does not produce a better matching between the experimental and the numerical results. (author)

  16. The coupling between flame surface dynamics and species mass conservation in premixed turbulent combustion

    NASA Technical Reports Server (NTRS)

    Trouve, A.; Veynante, D.; Bray, K. N. C.; Mantel, T.

    1994-01-01

    Current flamelot models based on a description of the flame surface dynamics require the closure of two inter-related equations: a transport equation for the mean reaction progress variable, (tilde)c, and a transport equation for the flame surface density, Sigma. The coupling between these two equations is investigated using direct numerical simulations (DNS) with emphasis on the correlation between the turbulent fluxes of (tilde)c, bar(pu''c''), and Sigma, (u'')(sub S)Sigma. Two different DNS databases are used in the present work: a database developed at CTR by A. Trouve and a database developed by C. J. Rutland using a different code. Both databases correspond to statistically one-dimensional premixed flames in isotropic turbulent flow. The run parameters, however, are significantly different, and the two databases correspond to different combustion regimes. It is found that in all simulated flames, the correlation between bar(pu''c'') and (u'')(sub S)Sigma is always strong. The sign, however, of the turbulent flux of (tilde)c or Sigma with respect to the mean gradients, delta(tilde)c/delta(x) or delta(Sigma)/delta(x), is case-dependent. The CTR database is found to exhibit gradient turbulent transport of (tilde)c and Sigma, whereas the Rutland DNS features counter-gradient diffusion. The two databases are analyzed and compared using various tools (a local analysis of the flow field near the flame, a classical analysis of the conservation equation for (tilde)(u''c''), and a thin flame theoretical analysis). A mechanism is then proposed to explain the discrepancies between the two databases and a preliminary simple criterion is derived to predict the occurrence of gradient/counter-gradient turbulent diffusion.

  17. EFFECTS OF EQUIVALENCE RATIO ON SPECIES AND SOOT CONCENTRATIONS IN PREMIXED N-HEPTANE FLAMES. (R828193)

    EPA Science Inventory

    The micro-structure of laminar premixed, atmospheric-pressure, fuel-rich flames of n-heptane/oxygen/argon has been studied at two equivalence ratios (C/O = 0.63 and C/O = 0.67). A heated quartz microprobe coupled to an online gas chromatography/mass spectrometry (HP 5890 Serie...

  18. THE EFFECTS OF EQUIVALENCE RATIO ON THE FORMATION OF POLYCYCLIC AROMATIC HYDROCARBONS AND SOOT IN PREMIXED ETHANE FLAMES. (R825412)

    EPA Science Inventory

    Abstract

    The formation of polycyclic aromatic hydrocarbons (PAH) and soot has been investigated in atmospheric-pressure, laminar, ethane/oxygen/argon premixed flames as a function of mixture equivalence ratio. Mole fraction profiles of major products, trace aromatics, ...

  19. An experimental study of the effect of a pilot flame on technically pre-mixed, self-excited combustion instabilities

    NASA Astrophysics Data System (ADS)

    O'Meara, Bridget C.

    Combustion instabilities are a problem facing the gas turbine industry in the operation of lean, pre-mixed combustors. Secondary flames known as "pilot flames" are a common passive control strategy for eliminating combustion instabilities in industrial gas turbines, but the underlying mechanisms responsible for the pilot flame's stabilizing effect are not well understood. This dissertation presents an experimental study of a pilot flame in a single-nozzle, swirl-stabilized, variable length atmospheric combustion test facility and the effect of the pilot on combustion instabilities. A variable length combustor tuned the acoustics of the system to excite instabilities over a range of operating conditions without a pilot flame. The inlet velocity was varied from 25 -- 50 m/s and the equivalence ratio was varied from 0.525 -- 0.65. This range of operating conditions was determined by the operating range of the combustion test facility. Stability at each operating condition and combustor length was characterized by measurements of pressure oscillations in the combustor. The effect of the pilot flame on the magnitude and frequency of combustor stability was then investigated. The mechanisms responsible for the pilot flame effect were studied using chemiluminescence flame images of both stable and unstable flames. Stable flame structure was investigated using stable flame images of CH* chemiluminescence emission. The effect of the pilot on stable flame metrics such as flame length, flame angle, and flame width was investigated. In addition, a new flame metric, flame base distance, was defined to characterize the effect of the pilot flame on stable flame anchoring of the flame base to the centerbody. The effect of the pilot flame on flame base anchoring was investigated because the improved stability with a pilot flame is usually attributed to improved flame anchoring through the recirculation of hot products from the pilot to the main flame base. Chemiluminescence images

  20. Combustion characteristics of pulverized coal and air/gas premixed flame in a double swirl combustor

    SciTech Connect

    Kamal, M.M.

    2009-07-01

    An experimental work was performed to investigate the co-firing of pulverized coal and premixed gas/air streams in a double swirl combustor. The results showed that the NOx emissions are affected by the relative rates of thermal NOx formation and destruction via the pyrolysis of the fuel-N species in high temperature fuel-rich zones. Various burner designs were tested in order to vary the temperature history and the residence time across both coal and gas flames inside the furnace. It was found that by injecting the coal with a gas/air mixture as a combined central jet surrounded by a swirled air stream, a double flame envelope develops with high temperature fuel-rich conditions in between the two reaction zones such that the pyrolysis reactions to N{sub 2} are accelerated. A further reduction in the minimum NOx emissions, as well as in the minimum CO concentrations, was reported for the case where the coal particles are fed with the gas/air mixture in the region between the two swirled air streams. On the other hand, allocating the gas/air mixture around the swirled air-coal combustion zone provides an earlier contact with air and retards the NOx reduction mechanism in such a way that the elevated temperatures around the coal particles allow higher overall NOx emissions. The downstream impingement of opposing air jets was found more efficient than the impinging of particle non-laden premixed flames for effective NOx reduction. In both cases, there is an upstream flow from the stagnation region to the coal primary combustion region, but with the case of air impingement, the hot fuel-rich zone develops earlier. The optimum configuration was found by impinging all jets of air and coal-gas/air mixtures that pronounced minimum NOx and CO concentrations of 310 and 480ppm, respectively.

  1. The structure and stability of the laminar counter-flow partially premixed methane/air triple flame

    SciTech Connect

    Lockett, R.D.; Boulanger, B.; Harding, S.C.; Greenhalgh, D.A.

    1999-10-01

    The flame stability map defining the regime of existence of a counter-flowing laminar partially premixed methane-air triple flame has been determined using OH planar laser-induced fluorescence (PLIF). The stability limits were determined through the observation of flame merging and flame extinction, a function of rich and lean equivalence ratios, and mean axial strain rate. Relatively quantitative OH species profiles and Rayleigh scattering profiles have been measured for three flame conditions. Axial flow velocity profiles, and nozzle exit velocity profiles have been determined for two of the three conditions using 1-D laser Doppler velocimetry (LDV). The diffusion flame extinction axial velocity profile has been measured, and the local extinction axial strain rate has been determined to be 710 s{sup {minus}1}.

  2. Numerical investigation of flame-vortex interactions in laminar cross-flow non-premixed flames in the presence of bluff bodies

    NASA Astrophysics Data System (ADS)

    Kozhumal Shijin, Puthiyaparambath; Raghavan, Vasudevan; Babu, Viswanathan

    2016-07-01

    Flame stabilisation in a combustor having vortices generated by flame holding devices constitutes an interesting fundamental problem. The presence of vortices in many practical combustors ranging from industrial burners to high speed propulsion systems induces vortex-flame interactions and complex stabilisation conditions. The scenario becomes more complex if the flame sustains after separating itself from the flame holder. In a recent study [P.K. Shijin, S.S. Sundaram, V. Raghavan, and V. Babu, Numerical investigation of laminar cross-flow non-premixed flames in the presence of a bluff-body, Combust. Theory Model. 18, 2014, pp. 692-710], the authors reported details of the regimes of flame stabilisation of non-premixed laminar flames established in a cross-flow combustor in the presence of a square cylinder. In that, the separated flame has been shown to be three dimensional and highly unsteady. Such separated flames are investigated further in the present study. Flame-vortex interactions in separated methane-air cross flow flames established behind three bluff bodies, namely a square cylinder, an isosceles triangular cylinder and a half V-gutter, have been analysed in detail. The mixing process in the reactive flow has been explained using streamlines of species velocities of CH4 and O2. The time histories of z-vorticity, net heat release rate and temperature are analysed to reveal the close relationship between z-vorticity and net heat release rate spectra. Two distinct fluctuating layers are visible in the proper orthogonal decomposition and discrete Fourier transform of OH mass fraction data. The upper fluctuating layer observed in the OH field correlates well with that of temperature. A detailed investigation of the characteristics of OH transport has also been carried out to show the interactions between factors affecting fluid dynamics and chemical kinetics that cause multiple fluctuating layers in the OH.

  3. A two-step chemical scheme for kerosene-air premixed flames

    SciTech Connect

    Franzelli, B.; Riber, E.; Sanjose, M.; Poinsot, T.

    2010-07-15

    A reduced two-step scheme (called 2S-KERO-BFER) for kerosene-air premixed flames is presented in the context of Large Eddy Simulation of reacting turbulent flows in industrial applications. The chemical mechanism is composed of two reactions corresponding to the fuel oxidation into CO and H{sub 2}O, and the CO - CO{sub 2} equilibrium. To ensure the validity of the scheme for rich combustion, the pre-exponential constants of the two reactions are tabulated versus the local equivalence ratio. The fuel and oxidizer exponents are chosen to guarantee the correct dependence of laminar flame speed with pressure. Due to a lack of experimental results, the detailed mechanism of Dagaut composed of 209 species and 1673 reactions, and the skeletal mechanism of Luche composed of 91 species and 991 reactions have been used to validate the reduced scheme. Computations of one-dimensional laminar flames have been performed with the 2S{sub K}ERO{sub B}FER scheme using the CANTERA and COSILAB softwares for a wide range of pressure ([1; 12] atm), fresh gas temperature ([300; 700] K), and equivalence ratio ([0.6; 2.0]). Results show that the flame speed is correctly predicted for the whole range of parameters, showing a maximum for stoichiometric flames, a decrease for rich combustion and a satisfactory pressure dependence. The burnt gas temperature and the dilution by Exhaust Gas Recirculation are also well reproduced. Moreover, the results for ignition delay time are in good agreement with the experiments. (author)

  4. Exploring old and new benzene formation pathways in low-pressure premixed flames of aliphatic fuels

    SciTech Connect

    Christopher J. Pope; James A. Miller

    2000-12-13

    A modeling study of benzene and phenyl radical formation is performed for three low-pressure premixed laminar flat flames having an unsaturated C{sub 2} or C{sub 3} hydrocarbon fuel (acetylene, ethylene, and propene). Predictions using three published detailed elementary-step chemical kinetics mechanisms are tested against MBMS species profile data for all three flames. The differences between the three mechanisms predictive capabilities are explored, with an emphasis on benzene formation pathways. A new chemical kinetics mechanism is created combining features of all three published mechanisms. Included in the mechanism are several novel benzene formation reactions involving combinations of radicals such as C{sub 2}H+C{sub 4}H{sub 5}, and C{sub 5}H{sub 3}+CH{sub 3}. Reactions forming fulvene (a benzene isomer) are included, such as C{sub 3}H{sub 3}+C{sub 3}H{sub 5},as well as fulvene-to-benzene reactions. Predictions using the new mechanism show virtually all of the benzene and phenyl radical to be formed by reactions of either C{sub 3}H{sub 3}+C{sub 3}H{sub 3} or C{sub 3}H{sub 3}+C{sub 3}H{sub 5}, with the relative importance being strongly dependent upon the fuel. C{sub 5}H{sub 3}+CH{sub 3} plays a minor role in fulvene formation in the acetylene flame. The C{sub 2}H{sub x}+C{sub 4}H{sub 4} reactions do not contribute noticeably to benzene or phenyl radical formation in these flames, sometimes being a major decomposition channel for either fulvene or phenyl radical. The formation pathways for C{sub 3}H{sub 3} and C{sub 3}H{sub 5}are delineated for the three flames; while the key reactions differ from flame to flame, CH{sub 2}+C{sub 2}H{sub 2} {Longleftrightarrow} C{sub 3}H{sub 3}+H is important for all three flames.

  5. Measurements of soot formation and hydroxyl concentration in near critical equivalence ratio premixed ethylene flame

    NASA Technical Reports Server (NTRS)

    Inbody, Michael Andrew

    1993-01-01

    The testing and development of existing global and detailed chemical kinetic models for soot formation requires measurements of soot and radical concentrations in flames. A clearer understanding of soot particle inception relies upon the evaluation and refinement of these models in comparison with such measurements. We present measurements of soot formation and hydroxyl (OH) concentration in sequences of flat premixed atmospheric-pressure C2H4/O2/N2 flames and 80-torr C2H4/O2 flames for a unique range of equivalence ratios bracketting the critical equivalence ratio (phi(sub c)) and extending to more heavily sooting conditions. Soot volume fraction and number density profiles are measured using a laser scattering-extinction apparatus capable of resolving a 0.1 percent absorption. Hydroxyl number density profiles are measured using laser-induced fluorescence (LIF) with broadband detection. Temperature profiles are obtained from Rayleigh scattering measurements. The relative volume fraction and number density profiles of the richer sooting flames exhibit the expected trends in soot formation. In near-phi(sub c) visibility sooting flames, particle scattering and extinction are not detected, but an LIF signal due to polycyclic aromatic hydrocarbons (PAH's) can be detected upon excitation with an argon-ion laser. A linear correlation between the argon-ion LIF and the soot volume fraction implies a common mechanistic source for the growth of PAH's and soot particles. The peak OH number density in both the atmospheric and 80-torr flames declines with increasing equivalence ratio, but the profile shape remains unchanged in the transition to sooting, implying that the primary reaction pathways for OH remain unchanged over this transition. Chemical kinetic modeling is demonstrated by comparing predictions using two current reaction mechanisms with the atmospheric flame data. The measured and predicted OH number density profiles show good agreement. The predicted benzene

  6. Measurements of the heat release rate integral in turbulent premixed stagnation flames with particle image velocimetry

    SciTech Connect

    Chen, Yung-Cheng; Kim, Munki; Han, Jeongjae; Yun, Sangwook; Yoon, Youngbin

    2008-08-15

    A new definition of turbulent consumption speed is proposed in this work that is based on the heat release rate integral, rather than the mass burning rate integral. Its detailed derivation and the assumptions involved are discussed in a general context that applies to all properly defined reaction progress variables. The major advantage of the proposed definition is that it does not require the thin-flame assumption, in contrast to previous definitions. Experimental determination of the local turbulent displacement speed, S{sub D}, and the local turbulent consumption speed, S{sub C}, is also demonstrated with the particle image velocimetry technique in three turbulent premixed stagnation flames. The turbulence intensity of these flames is of the same order of the laminar burning velocity. Based on the current data, a model equation for the local mean heat release rate is proposed. The relationship between S{sub D} and S{sub C} is discussed along with a possible modeling approach for the turbulent displacement speed. (author)

  7. Lagrangian Fluid Element Tracking and Estimation of Local Displacement Speeds in Turbulent Premixed Flames

    NASA Astrophysics Data System (ADS)

    Ramji, Sarah Ann

    Improved understanding of turbulence-flame interactions in premixed combustion can be achieved using fully 3D time-resolved multi-kHz multi-scalar experimental measurements. These interactions may be represented by the evolution of various Lagrangian quantities described by theoretical Lagrangian Fluid Elements (LFEs). The data used in this work came from two experimental campaigns that used simultaneous T-PIV and OH/CH2O PLIF, at Sandia National Labs and the Air Force Research Lab at Wright-Patterson. In this thesis, an algorithm to accurately track LFEs through this 4D experimental space has been developed and verified by cross-correlation with the T-PIV seed particle fields. A novel method to measure the local instantaneous displacement speed in 3D has been developed, using this algorithm to track control masses of fluid that interact with the flame front. Statistics of the displacement speed have been presented, and the effects of local turbulence and flame topological properties on the displacement speed have been studied.

  8. A Study of Strain Rate Effects for Turbulent Premixed Flames with Application to LES of a Gas Turbine Combustor Model

    DOE PAGESBeta

    Kemenov, Konstantin A.; Calhoon, William H.

    2015-03-24

    Large-scale strain rate field, a resolved quantity which is easily computable in large-eddy simulations (LES), could have profound effects on the premixed flame properties by altering the turbulent flame speed and inducing local extinction. The role of the resolved strain rate has been investigated in a posterior LES study of GE lean premixed dry low NOx emissions LM6000 gas turbine combustor model. A novel approach which is based on the coupling of the lineareddy model with a one-dimensional counter-flow solver has been applied to obtain the parameterizations of the resolved premixed flame properties in terms of the reactive progress variable,more » the local strain rate measure, and local Reynolds and Karlovitz numbers. The strain rate effects have been analyzed by comparing LES statistics for several models of the turbulent flame speed, i.e, with and without accounting for the local strain rate effects, with available experimental data. The sensitivity of the simulation results to the inflow velocity conditions as well as the grid resolution have been also studied. Overall, the results suggest the necessity to represent the strain rate effects accurately in order to improve LES modeling of the turbulent flame speed.« less

  9. A Study of Strain Rate Effects for Turbulent Premixed Flames with Application to LES of a Gas Turbine Combustor Model

    SciTech Connect

    Kemenov, Konstantin A.; Calhoon, William H.

    2015-03-24

    Large-scale strain rate field, a resolved quantity which is easily computable in large-eddy simulations (LES), could have profound effects on the premixed flame properties by altering the turbulent flame speed and inducing local extinction. The role of the resolved strain rate has been investigated in a posterior LES study of GE lean premixed dry low NOx emissions LM6000 gas turbine combustor model. A novel approach which is based on the coupling of the lineareddy model with a one-dimensional counter-flow solver has been applied to obtain the parameterizations of the resolved premixed flame properties in terms of the reactive progress variable, the local strain rate measure, and local Reynolds and Karlovitz numbers. The strain rate effects have been analyzed by comparing LES statistics for several models of the turbulent flame speed, i.e, with and without accounting for the local strain rate effects, with available experimental data. The sensitivity of the simulation results to the inflow velocity conditions as well as the grid resolution have been also studied. Overall, the results suggest the necessity to represent the strain rate effects accurately in order to improve LES modeling of the turbulent flame speed.

  10. Magnifying and Tracking Observation of Micro PET Particles Passing through a Plane Premixed Flame Front

    NASA Astrophysics Data System (ADS)

    Ohiwa, Norio; Ishino, Yojiro; Tomatsu, Takanori; Yamakita, Ryuji

    In order to observe detailed behavior of micro plastic particles under rapid heating, a fundamental investigation is made by introducing two ingenious devices; one is the construction of a plane laminar premixed burner exhibiting extremely excellent two-dimensionality, the other is the construction of a magnifying particle-tracking system composed of a pair of rotating plane mirrors and a fixed high-speed video camera. Taking account of the flow patterns obtained using a PIV/PTV system, a series of heating processes from melting to burning of micro PET particles passing through a laminar flame sheet is optically observed. It is found that the proposed high-speed and magnifying tracking system can realize a wide straight range of particle tracking up to 50 mm and clarify many interesting facts concerning the ignition and burning processes of micro PET particles.

  11. LES-Modeling of a Partially Premixed Flame using a Deconvolution Turbulence Closure

    NASA Astrophysics Data System (ADS)

    Wang, Qing; Wu, Hao; Ihme, Matthias

    2015-11-01

    The modeling of the turbulence/chemistry interaction in partially premixed and multi-stream combustion remains an outstanding issue. By extending a recently developed constrained minimum mean-square error deconvolution (CMMSED) method, to objective of this work is to develop a source-term closure for turbulent multi-stream combustion. In this method, the chemical source term is obtained from a three-stream flamelet model, and CMMSED is used as closure model, thereby eliminating the need for presumed PDF-modeling. The model is applied to LES of a piloted turbulent jet flame with inhomogeneous inlets, and simulation results are compared with experiments. Comparisons with presumed PDF-methods are performed, and issues regarding resolution and conservation of the CMMSED method are examined. The author would like to acknowledge the support of funding from Stanford Graduate Fellowship.

  12. The multispecies modeling of the premixed, laminar steady-state ozone flame

    NASA Technical Reports Server (NTRS)

    Heimerl, J. M.; Coffee, T. P.

    1980-01-01

    Species dependent kinetic, transport and thermodynamic coefficients were employed in a one dimensional model of the premixed, laminar, steady state ozone flame. Convenient expressions for these coefficients are reported. They are based on independent measurements, no arbitrary parameters are used. The governing equations are solved using a relaxation technique and the partial differential equation package, PDECOL. Species and temperature profiles and the burning velocities are found over the range of initial ozone mole fraction of 0.25 to 1.00. The computed burning velocities are no more than 30% greater than the measurements of Streng and Grosses. Comparison with the computed results of Warnatz shows agreement within + or - 12%, even though quite different expressions for some of the kinetic coefficients were used. These differences are most obvious in the atomic oxygen and temperature profiles at an initial ozone mole fraction of unity.

  13. Conditional statistics in a turbulent premixed flame derived from direct numerical simulation

    NASA Technical Reports Server (NTRS)

    Mantel, Thierry; Bilger, Robert W.

    1994-01-01

    The objective of this paper is to briefly introduce conditional moment closure (CMC) methods for premixed systems and to derive the transport equation for the conditional species mass fraction conditioned on the progress variable based on the enthalpy. Our statistical analysis will be based on the 3-D DNS database of Trouve and Poinsot available at the Center for Turbulence Research. The initial conditions and characteristics (turbulence, thermo-diffusive properties) as well as the numerical method utilized in the DNS of Trouve and Poinsot are presented, and some details concerning our statistical analysis are also given. From the analysis of DNS results, the effects of the position in the flame brush, of the Damkoehler and Lewis numbers on the conditional mean scalar dissipation, and conditional mean velocity are presented and discussed. Information concerning unconditional turbulent fluxes are also presented. The anomaly found in previous studies of counter-gradient diffusion for the turbulent flux of the progress variable is investigated.

  14. Chemiluminescence-based multivariate sensing of local equivalence ratios in premixed atmospheric methane-air flames

    SciTech Connect

    Tripathi, Markandey M.; Krishnan, Sundar R.; Srinivasan, Kalyan K.; Yueh, Fang-Yu; Singh, Jagdish P.

    2011-09-07

    Chemiluminescence emissions from OH*, CH*, C2, and CO2 formed within the reaction zone of premixed flames depend upon the fuel-air equivalence ratio in the burning mixture. In the present paper, a new partial least square regression (PLS-R) based multivariate sensing methodology is investigated and compared with an OH*/CH* intensity ratio-based calibration model for sensing equivalence ratio in atmospheric methane-air premixed flames. Five replications of spectral data at nine different equivalence ratios ranging from 0.73 to 1.48 were used in the calibration of both models. During model development, the PLS-R model was initially validated with the calibration data set using the leave-one-out cross validation technique. Since the PLS-R model used the entire raw spectral intensities, it did not need the nonlinear background subtraction of CO2 emission that is required for typical OH*/CH* intensity ratio calibrations. An unbiased spectral data set (not used in the PLS-R model development), for 28 different equivalence ratio conditions ranging from 0.71 to 1.67, was used to predict equivalence ratios using the PLS-R and the intensity ratio calibration models. It was found that the equivalence ratios predicted with the PLS-R based multivariate calibration model matched the experimentally measured equivalence ratios within 7%; whereas, the OH*/CH* intensity ratio calibration grossly underpredicted equivalence ratios in comparison to measured equivalence ratios, especially under rich conditions ( > 1.2). The practical implications of the chemiluminescence-based multivariate equivalence ratio sensing methodology are also discussed.

  15. Experimental study of the stabilization process of a non-premixed flame via the destabilization analysis of the blue ring flame

    SciTech Connect

    Pinguet, Guillaume; Escudie, Dany

    2007-04-15

    The flame stabilization phenomenon remains a crucial issue. The experimental study of flame stabilization behind a tulip-shaped flame-holder is addressed in this paper. The process leading to the transition between specific modes - the blue ring flame and the instable ring - of a non-premixed flame stabilized on a tulip-shaped bluff-body is detailed. The aim of this study is to provide an accurate description of the destabilization of specific combustion modes, which enables a further understanding of the entire stabilization mechanism. The aerodynamic and mixing fields are described by laser Doppler anemometry and concentration measurements by sampling probe respectively. The behaviour of shear layers developing at the wake and jet boundaries are characterized by means of a spectral analysis of the fluctuating radial velocity. Results show that the destabilization process is related to the intensification of hot gas recirculation, inducing an upheaval of the dynamical condition of stabilization and a transition of mixing phenomena. (author)

  16. Optical measurements of soot and temperature profiles in premixed propane-oxygen flames

    NASA Technical Reports Server (NTRS)

    Lyons, Valerie J.; Pagni, Patrick J.

    1988-01-01

    Two laser diagnostic techniques were used to measure soot volume fractions, number densities and soot particle radii in premixed propane/oxygen flat flames. The two techniques used were two wavelength extinction, using 514.5 nm to 632.8 nm and 457.9 nm to 632.8 nm wavelength combinations, and extinction/scattering using 514.5 nm light. The flames wre fuel-rich (equivalence ratios from 2.1 to 2.8) and had cold gas velocities varying from 3.4 to 5.5 cm/s. Measurements were made at various heights above the sintered-bronze, water-cooled flat flame burner with the equivalence ratio and cold gas velocity fixed. Also, measurements were made at a fixed height above the burner and fixed cold gas velocity while varying the equivalence ratio. Both laser techniques are based on the same underlying assumptions of particle size distribution and soot optical properties. Full Mie theory was used to determine the extinction coefficients K sub ext, and the scattering efficiencies, Q sub vv. Temperature measurements in the flames were made using infrared radiometry. Good agreement between the two techniques in terms of soot particle radii, number density and volume fraction was found for intensity ratios (I/I sub o) between 0.1 and 0.8. For intensity ratios higher or lower than this range, the differences in extinction coefficients at the wavelengths chosen for the two-wavelength method are too small to give accurate results for comparing particle radii and number densities. However, when comparing only soot volume fractions, the agreement between the two techniques continued to be good for intensity ratios up to 0.95.

  17. Optical measurements of soot and temperature profiles in premixed propane-oxygen flames

    NASA Technical Reports Server (NTRS)

    Lyons, V. J.; Pagni, P. J.

    1988-01-01

    Two laser diagnostic techniques were used to measure soot volume fractions, number densities and soot particle radii in premixed propane/oxygen flat flames. The two techniques used were two wavelength extinction, using 514.5 nm to 632.8 nm and 457.9 nm to 632.8 nm wavelength combinations, and extinction/scattering using 514.5 nm light. The flames were fuel-rich (equivalence ratios from 2.1 to 2.8) and had cold gas velocities varying from 3.4 to 5.5 cm/s. Measurements were made at various heights above the sintered-bronze, water-cooled flat flame burner with the equivalence ratio and cold gas velocity fixed. Also, measurements were made at a fixed height above the burner and fixed cold gas velocity while varying the equivalence ratio. Both laser techniques are based on the same underlying assumptions of particle size distribution and soot optical properties. Full Mie theory was used to determine the extinction coefficients K sub ext, and the scattering efficiencies, Q sub vv. Temperature measurements in the flames were made using infrared radiometry. Good agreement between the two techniques in terms of soot particle radii, number density and volume fraction was found for intensity ratios (I/I sub o) between 0.1 and 0.8. For intensity ratios higher or lower than this range, the differences in extinction coefficients at the wavelengths chosen for the two-wavelength method are too small to give accurate results for comparing particle radii and number densities. However, when comparing only soot volume fractions, the agreement between the two techniques continued to be good for intensity ratios up to 0.95.

  18. Effects of Radiative Emission and Absorption on the Propagation and Extinction of Premixed Gas Flames

    NASA Technical Reports Server (NTRS)

    Ju, Yiguang; Masuya, Goro; Ronney, Paul D.

    1998-01-01

    Premixed gas flames in mixtures of CH4, O2, N2, and CO2 were studied numerically using detailed chemical and radiative emission-absorption models to establish the conditions for which radiatively induced extinction limits may exist independent of the system dimensions. It was found that reabsorption of emitted radiation led to substantially higher burning velocities and wider extinction limits than calculations using optically thin radiation models, particularly when CO2, a strong absorber, is present in the unburned gas, Two heat loss mechanisms that lead to flammability limits even with reabsorption were identified. One is that for dry hydrocarbon-air mixtures, because of the differences in the absorption spectra of H2O and CO2, most of the radiation from product H2O that is emitted in the upstream direction cannot be absorbed by the reactants. The second is that the emission spectrum Of CO2 is broader at flame temperatures than ambient temperature: thus, some radiation emitted near the flame front cannot be absorbed by the reactants even when they are seeded with CO2 Via both mechanisms, some net upstream heat loss due to radiation will always occur, leading to extinction of sufficiently weak mixtures. Downstream loss has practically no influence. Comparison with experiment demonstrates the importance of reabsorption in CO2 diluted mixtures. It is concluded that fundamental flammability limits can exist due to radiative heat loss, but these limits are strongly dependent on the emission-absorption spectra of the reactant and product -gases and their temperature dependence and cannot be predicted using gray-gas or optically thin model parameters. Applications to practical flames at high pressure, in large combustion chambers, and with exhaust-gas or flue-gas recirculation are discussed.

  19. Enhancement of a laminar premixed methane/oxygen/nitrogen flame speed using femtosecond-laser-induced plasma

    SciTech Connect

    Yu Xin; Peng Jiangbo; Yi Yachao; Zhao Yongpeng; Chen Deying; Yu Junhua; Yang Peng; Sun Rui

    2010-07-05

    We first investigate the effects of femtosecond-laser-induced plasma on the flame speed of a laminar premixed methane/oxygen/nitrogen flame with a wide range of the equivalence ratios (0.8-1.05) at atmospheric pressure. It is experimentally found that the flame speed increases 20.5% at equivalence ratios 1.05. The self-emission spectra from the flame and the plasma are studied and an efficient production of active radicals under the action of femtosecond (fs)-laser pulses has been observed. Based on the experimental data obtained, the presence of oxygen atom and hydrocarbon radicals is suggested to be a key factor enhancing flame speed.

  20. Cellular burning in lean premixed turbulent hydrogen-air flames: Coupling experimental and computational analysis at the laboratory scale

    NASA Astrophysics Data System (ADS)

    Day, M. S.; Bell, J. B.; Cheng, R. K.; Tachibana, S.; Beckner, V. E.; Lijewski, M. J.

    2009-07-01

    One strategy for reducing US dependence on petroleum is to develop new combustion technologies for burning the fuel-lean mixtures of hydrogen or hydrogen-rich syngas fuels obtained from the gasification of coal and biomass. Fuel-flexible combustion systems based on lean premixed combustion have the potential for dramatically reducing pollutant emissions in transportation systems, heat and stationary power generation. However, lean premixed flames are highly susceptible to fluid-dynamical combustion instabilities making robust and reliable systems difficult to design. Low swirl burners are emerging as an important technology for meeting design requirements in terms of both reliability and emissions for next generation combustion devices. In this paper, we present simulations of a lean, premixed hydrogen flame stabilized on a laboratory-scale low swirl burner. The simulations use detailed chemistry and transport without incorporating explicit models for turbulence or turbulence/chemistry interaction. Here we discuss the overall structure of the flame and compare with experimental data. We also use the simulation data to elucidate the characteristics of the turbulent flame interaction and how this impacts the analysis of experimental measurements.

  1. Study on the Enhancement Effect of Dielectric Barrier Discharge on the Premixed Methane/Oxygen/Helium Flame Velocity

    NASA Astrophysics Data System (ADS)

    Mu, Haibao; Yu, Lin; Li, Ping; Tang, Chenglong; Wang, Jinhua; Zhang, Guanjun

    2015-12-01

    Recently, plasma-assisted combustion has become a potentially applicable technology in many combustion scenarios. In this paper, a dielectric barrier discharge (DBD) plasma generator is designed to explore the effect of plasma on the CH4 oxidation process, and several properties of combustion are considered. First, in the presence or absence of plasma discharge, physical appearance of the flame is examined and analyzed. Second, the flame propagation velocity is calculated by the flame front extracted from the imaging data with the Bunsen burner method. Finally, the main molecular components and their intensity variation in the flame and the plasma zones are identified with an emission spectrograph to analyze the effect of active species on the combustion process. We also discuss the possible kinetic regime of plasma-assisted combustion. Experimental results imply that plasma discharge applied to the premixed CH4/O2/He mixture significantly raises the flame speed with equivalence ratios ranging from 0.85 to 1.10, with the flame speed improved by 17% to 35%. It can be seen that plasma can improve methane oxidation efficiency in the premixed fuel/oxidizer, especially at a low equivalence ratio. supported by the Fundamental Research Funds for the Central Universities of China (No. xjj2013086), Natural Science Basic Research Plan in Shaanxi Province of China (No. 2014JQ7254) and National Natural Science Foundation of China (No. 51477135)

  2. Numerical prediction of turbulent flame stability in premixed/prevaporized (HSCT) combustors

    NASA Technical Reports Server (NTRS)

    Winowich, Nicholas S.

    1990-01-01

    A numerical analysis of combustion instabilities that induce flashback in a lean, premixed, prevaporized dump combustor is performed. KIVA-II, a finite volume CFD code for the modeling of transient, multidimensional, chemically reactive flows, serves as the principal analytical tool. The experiment of Proctor and T'ien is used as a reference for developing the computational model. An experimentally derived combustion instability mechanism is presented on the basis of the observations of Proctor and T'ien and other investigators of instabilities in low speed (M less than 0.1) dump combustors. The analysis comprises two independent procedures that begin from a calculated stable flame: The first is a linear increase of the equivalence ratio and the second is the linear decrease of the inflow velocity. The objective is to observe changes in the aerothermochemical features of the flow field prior to flashback. It was found that only the linear increase of the equivalence ratio elicits a calculated flashback result. Though this result did not exhibit large scale coherent vortices in the turbulent shear layer coincident with a flame flickering mode as was observed experimentally, there were interesting acoustic effects which were resolved quite well in the calculation. A discussion of the k-e turbulence model used by KIVA-II is prompted by the absence of combustion instabilities in the model as the inflow velocity is linearly decreased. Finally, recommendations are made for further numerical analysis that may improve correlation with experimentally observed combustion instabilities.

  3. Effects of Lewis number, density ratio and gravity on burning velocity and conditional statistics in stagnating turbulent premixed flames

    NASA Astrophysics Data System (ADS)

    Kwon, Jaesung; Huh, Kang Y.

    2014-09-01

    DNS is performed to analyse the effects of Lewis number (Le), density ratio and gravity in stagnating turbulent premixed flames. The results show good agreement with those of Lee and Huh (Combustion and Flame, Vol. 159, 2012, pp. 1576-1591) with respect to the turbulent burning velocity, ST, in terms of turbulent diffusivity, flamelet thickness, mean curvature and displacement speed at the leading edge. In all four stagnating flames studied, a mean tangential strain rate resulting in a mean flamelet thickness smaller than the unstretched laminar flame thickness leads to an increase in ST. A flame cusp of positive curvature involves a superadiabatic burned gas temperature due to diffusive-thermal instability for an Le less than unity. Wrinkling tends to be suppressed at a larger density ratio, not enhanced by hydrodynamic instability, in the stagnating flow configuration. Turbulence is produced, resulting in highly anisotropic turbulence with heavier unburned gas accelerating through a flame brush by Rayleigh-Taylor instability. Results are also provided on brush thickness, flame surface density and conditional velocities in burned and unburned gas and on flame surfaces to represent the internal brush structures for all four test flames.

  4. Rich premixed laminar methane flames doped by light unsaturated hydrocarbons. II. 1,3-Butadiene

    SciTech Connect

    Gueniche, H.A.; Glaude, P.A.; Fournet, R.; Battin-Leclerc, F.

    2007-10-15

    In line with the study presented in Part I of this paper, the structure of a rich premixed laminar methane flame doped with 1,3-butadiene has been investigated. The flame contains 20.7% (molar) of methane, 31.4% of oxygen, and 3.3% of 1,3-butadiene, corresponding to an equivalence ratio of 1.8, and a C{sub 4}H{sub 6}/CH{sub 4} ratio of 16%. The flame has been stabilized on a burner at a pressure of 6.7 kPa using argon as dilutant, with a gas velocity at the burner of 36 cm/s at 333 K. The temperature ranged from 600 K close to the burner up to 2150 K. Quantified species included the usual methane C{sub 0}-C{sub 2} combustion products and 1,3-butadiene, but also propyne, allene, propene, propane, 1,2-butadiene, butynes, vinylacetylene, diacetylene, 1,3-pentadiene, 2-methyl-1,3-butadiene (isoprene), 1-pentene, 3-methyl-1-butene, benzene, and toluene. To model these new results, some improvements have been made to a mechanism previously developed in our laboratory for the reactions of C{sub 3}-C{sub 4} unsaturated hydrocarbons. The main reaction pathways of consumption of 1,3-butadiene and of formation of C{sub 6} aromatic species have been derived from flow rate analyses. In this case, the C{sub 4} route to benzene formation plays an important role in comparison to the C{sub 3} pathway. (author)

  5. Experimental data regarding the characterization of the flame behavior near lean blowout in a non-premixed liquid fuel burner

    PubMed Central

    De Giorgi, Maria Grazia; Sciolti, Aldebara; Campilongo, Stefano; Ficarella, Antonio

    2015-01-01

    The article presents the data related to the flame acquisitions in a liquid-fuel gas turbine derived burner operating in non-premixed mode under three different equivalence fuel/air ratio, which corresponds to a richer, an intermediate, and an ultra-lean condition, near lean blowout (LBO). The data were collected with two high speed visualization systems which acquired in the visible (VIS) and in the infrared (NIR) spectral region. Furthermore chemiluminescence measurements, which have been performed with a photomultiplier (PMT), equipped with an OH* filter, and gas exhaust measurements were also given. For each acquisition the data were related to operating parameters as pressure, temperature and equivalent fuel/air ratio. The data are related to the research article “Image processing for the characterization of flame stability in a non-premixed liquid fuel burner near lean blowout” in Aerospace Science and Technology [1]. PMID:26862557

  6. Experimental data regarding the characterization of the flame behavior near lean blowout in a non-premixed liquid fuel burner.

    PubMed

    De Giorgi, Maria Grazia; Sciolti, Aldebara; Campilongo, Stefano; Ficarella, Antonio

    2016-03-01

    The article presents the data related to the flame acquisitions in a liquid-fuel gas turbine derived burner operating in non-premixed mode under three different equivalence fuel/air ratio, which corresponds to a richer, an intermediate, and an ultra-lean condition, near lean blowout (LBO). The data were collected with two high speed visualization systems which acquired in the visible (VIS) and in the infrared (NIR) spectral region. Furthermore chemiluminescence measurements, which have been performed with a photomultiplier (PMT), equipped with an OH* filter, and gas exhaust measurements were also given. For each acquisition the data were related to operating parameters as pressure, temperature and equivalent fuel/air ratio. The data are related to the research article "Image processing for the characterization of flame stability in a non-premixed liquid fuel burner near lean blowout" in Aerospace Science and Technology [1].

  7. Experimental data regarding the characterization of the flame behavior near lean blowout in a non-premixed liquid fuel burner.

    PubMed

    De Giorgi, Maria Grazia; Sciolti, Aldebara; Campilongo, Stefano; Ficarella, Antonio

    2016-03-01

    The article presents the data related to the flame acquisitions in a liquid-fuel gas turbine derived burner operating in non-premixed mode under three different equivalence fuel/air ratio, which corresponds to a richer, an intermediate, and an ultra-lean condition, near lean blowout (LBO). The data were collected with two high speed visualization systems which acquired in the visible (VIS) and in the infrared (NIR) spectral region. Furthermore chemiluminescence measurements, which have been performed with a photomultiplier (PMT), equipped with an OH* filter, and gas exhaust measurements were also given. For each acquisition the data were related to operating parameters as pressure, temperature and equivalent fuel/air ratio. The data are related to the research article "Image processing for the characterization of flame stability in a non-premixed liquid fuel burner near lean blowout" in Aerospace Science and Technology [1]. PMID:26862557

  8. Combustion Characteristics in a Non-Premixed Cool-Flame Regime of n-Heptane in Microgravity

    NASA Technical Reports Server (NTRS)

    Takahashi, Fumiaki; Katta, Viswanath R.; Hicks, Michael C.

    2015-01-01

    A series of distinct phenomena have recently been observed in single-fuel-droplet combustion tests performed on the International Space Station (ISS). This study attempts to simulate the observed flame behavior numerically using a gaseous n-heptane fuel source in zero gravity and a time-dependent axisymmetric (2D) code, which includes a detailed reaction mechanism (127 species and 1130 reactions), diffusive transport, and a radiation model (for CH4, CO, CO2, H2O, and soot). The calculated combustion characteristics depend strongly on the air velocity around the fuel source. In a near-quiescent air environment (< or = 2 mm/s), with a sufficiently large fuel injection velocity (1 cm/s), a growing spherical diffusion flame extinguishes at ˜1200 K due to radiative heat losses. This is typically followed by a transition to the low-temperature (cool-flame) regime with a reaction zone (at ˜700 K) in close proximity to the fuel source. The 'cool flame' regime is formed due to the negative temperature coefficient in the low-temperature chemistry. After a relatively long period (˜18 s) of the cool flame regime, a flash re-ignition occurs, associated with flame-edge propagation and subsequent extinction of the re-ignited flame. In a low-speed (˜3 mm/s) airstream (which simulates the slight droplet movement), the diffusion flame is enhanced upstream and experiences a local extinction downstream at ˜1200 K, followed by steady flame pulsations (˜0.4 Hz). At higher air velocities (4-10 mm/s), the locally extinguished flame becomes steady state. The present axisymmetric computational approach helps in revealing the non-premixed 'cool flame' structure and 2D flame-flow interactions observed in recent microgravity droplet combustion experiments.

  9. The mechanism of two-dimensional pocket formation in lean premixed methane-air flames with implications to turbulent combustion

    SciTech Connect

    Chen, J.H.; Echekki, T.; Kollmann, W.

    1999-01-01

    The mechanism of unburnt pocket formation in an unsteady two-dimensional premixed lean methane-air flame is investigated using direct numerical simulations. Theoretical results for nonlinear diffusion equations combined with analytical examples are used to interpret some of the results. Flame structure and propagation show three distinct stages of pocket formation: (1) flame channel closing involving head-on quenching of flames, (2) cusp recovery, and (3) pocket burnout. The flame channel closing and subsequent pocket burnout are mutual annihilation events that feature curvature, diffusion normal to the flame front, unsteady strain rate effects, and singularities in flame propagation and stretch rate. The results show that during channel closing and pocket burnout thermo-diffusive and chemical interactions result in the acceleration of the flames prior to annihilation; the time scales associated with the final stage of mutual annihilation and the initial stage of cusp recovery are significantly smaller than diffusive and convective time scales. Peak radical concentrations resulting from flame channel closing and pocket burnout exceed peak laminar values by as much as 25%. After the merging of the fuel consumption layers, radical production and flame structure shifts more towards an H{sub 2}/CO/O{sub 2} system at the expense of hydrocarbon reactions. Species thermodiffusive interaction times are shorter than the unstrained one-dimensional counterpart due to unsteady strain and convection. Curvature effects on the flame propagation are prominent during pocket burnout and cusp recovery. The recovery stage shows strong dependence on diffusion of radicals left from the channel closing stage. This diffusion is amplified by the strong curvature of the flame cusp.

  10. High-temperature oxidation chemistry of n-butanol--experiments in low-pressure premixed flames and detailed kinetic modeling.

    PubMed

    Hansen, N; Harper, M R; Green, W H

    2011-12-01

    An automated reaction mechanism generator is used to develop a predictive, comprehensive reaction mechanism for the high-temperature oxidation chemistry of n-butanol. This new kinetic model is an advancement of an earlier model, which had been extensively tested against earlier experimental data (Harper et al., Combust. Flame, 2011, 158, 16-41). In this study, the model's predictive capabilities are improved by targeting isomer-resolved quantitative mole fraction profiles of flame species in low-pressure flames. To this end, a total of three burner-stabilized premixed flames are isomer-selectively analyzed by flame-sampling molecular-beam time-of-flight mass spectrometry using photoionization by tunable vacuum-ultraviolet synchrotron radiation. For most species, the newly developed chemical kinetic model is capable of accurately reproducing the experimental trends in these flames. The results clearly indicate that n-butanol is mainly consumed by H-atom abstraction with H, O, and OH, forming predominantly the α-C(4)H(9)O radical (CH(3)CH(2)CH(2)˙CHOH). Fission of C-C bonds in n-butanol is only predicted to be significant in a similar, but hotter flame studied by Oßwald et al. (Combust. Flame, 2011, 158, 2-15). The water-elimination reaction to 1-butene is found to be of no importance under the premixed conditions studied here. The initially formed isomeric C(4)H(9)O radicals are predicted to further oxidize by reacting with H and O(2) or to decompose to smaller fragments via β-scission. Enols are detected experimentally, with their importance being overpredicted by the model. PMID:21993635

  11. Blowoff characteristics of bluff-body stabilized conical premixed flames with upstream spatial mixture gradients and velocity oscillations

    SciTech Connect

    Chaudhuri, Swetaprovo; Cetegen, Baki M.

    2008-06-15

    This experimental study concerns determination of blowoff equivalence ratios for lean premixed conical flames for different mixture approach velocities ranging from 5 to 16 m/s in the presence of spatial mixture gradients and upstream velocity modulation. Conical flames were anchored on a disk-shaped bluff body that was attached to a central rod in the burner nozzle. A combustible propane-air mixture flowed through a converging axisymmetric nozzle with a concentric insert, allowing radial mixture variation by tailoring the composition in the inner and outer parts of the nozzle. The radial mixture profiles were characterized near the location of the flame holder by laser Rayleigh light scattering. Additionally, a loudspeaker at the nozzle base allowed introduction of periodic velocity oscillations with an amplitude of 9% of the mean flow velocity up to a frequency of 350 Hz. The flame blowoff equivalence ratio was experimentally determined by continuously lowering the fuel flow rates and determining the flame detachment point from the flame holder. Flame detachment was detected by a rapid reduction of CH* emission from the flame base imaged by a photomultiplier detector. It was found that the flame blowoff is preceded by progressive narrowing of the flame cone for the case of higher inner jet equivalence ratios. In this case, the fuel-lean outer flow cannot sustain combustion, and clearly this is not a good way of operating a combustor. Nevertheless, the overall blowoff equivalence ratio is reduced by inner stream fuel enrichment. A possible explanation for this behavior is given based on the radial extent of the variable-equivalence-ratio mixture burning near the flame stabilization region. Fuel enrichment in the outer flow was found to have no effect on blowoff as compared to the case of uniform mixture. The results were similar for the whole range of mean flow velocities and upstream excitation frequencies. (author)

  12. Dynamics and Structure of Dusty Reacting Flows: Inert Particles in Strained, Laminar, Premixed Flames

    NASA Technical Reports Server (NTRS)

    Egolfopoulos, Fokion N.; Campbell, Charles S.; Wu, Ming-Shin (Technical Monitor)

    1999-01-01

    A detailed numerical study was conducted on the dynamics and thermal response of inert spherical particles in strained, laminar, premixed hydrogen/air flames. The modeling included the solution of the steady conservation equations for both the gas and particle phases along and around the stagnation streamline of an opposed-jet configuration, and the use of detailed descriptions of chemical kinetics and molecular transport. For the gas phase, the equations of mass, momentum, energy, and species are considered, while for the particle phase, the model is based on conservation equations of the particle momentum balance in the axial and radial direction, the particle number density, and the particle thermal energy equation. The particle momentum equation includes the forces as induced by drag, thermophoresis, and gravity. The particle thermal energy equation includes the convective/conductive heat exchange between the two phases, as well as radiation emission and absorption by the particle. A one-point continuation method is also included in the code that allows for the description of turning points, typical of ignition and extinction behavior. As expected, results showed that the particle velocity can be substantially different than the gas phase velocity, especially in the presence of large temperature gradients and large strain rates. Large particles were also found to cross the gas stagnation plane, stagnate, and eventually reverse as a result of the opposing gas phase velocity. It was also shown that the particle number density varies substantially throughout the flowfield, as a result of the straining of the flow and the thermal expansion. Finally, for increased values of the particle number density, substantial flame cooling to extinction states and modification of the gas phase fluid mechanics were observed. As also expected, the effect of gravity was shown to be important for low convective velocities and heavy particles. Under such conditions, simulations

  13. Dynamics and Structure of Dusty Reacting Flows: Inert Particles in Strained, Laminar, Premixed Flames

    NASA Technical Reports Server (NTRS)

    Egolfopoulos, Fokion N.; Campbell, Charles S.

    1999-01-01

    A detailed numerical study was conducted on the dynamics and thermal response of inert, spherical particles in strained, laminar, premixed hydrogen/air flames. The modeling included the solution of the steady conservation equations for both the gas and particle phases along and around the stagnation streamline of an opposed-jet configuration, and the use of detailed descriptions of chemical kinetics and molecular transport, For the gas phase, the equations of mass, momentum, energy, and species are considered, while for the particle phase, the model is based on conservation equations of the particle momentum balance in the axial and radial direction, the particle number density, and the particle thermal energy equation. The particle momentum equation includes the forces as induced by drag, thermophoresis, and gravity. The particle thermal energy equation includes the convective/conductive heat exchange between the two phases, as well as radiation emission and absorption by the particle. A one-point continuation method is also included in the code that allows for the description of turning points, typical of ignition and extinction behavior. As expected, results showed that the particle velocity can be substantially different than the gas phase velocity, especially in the presence of large temperature gradients and large strain rates. Large particles were also found to cross the gas stagnation plane, stagnate, and eventually reverse as a result of the opposing gas phase velocity. It was also shown that the particle number density varies substantially throughout the flowfield, as a result of the straining of the flow and the thermal expansion. Finally, for increased values of the particle number density, substantial flame cooling to extinction states and modification of the gas phase fluid mechanics were observed. As also expected, the effect of gravity was shown to be important for low convective velocities and heavy particles. Under such conditions, simulations

  14. Large Eddy Simulations of forced ignition of a non-premixed bluff-body methane flame with Conditional Moment Closure

    SciTech Connect

    Triantafyllidis, A.; Mastorakos, E.; Eggels, R.L.G.M.

    2009-12-15

    Large Eddy Simulations (LES) of forced ignition of a bluff-body stabilised non-premixed methane flame using the Conditional Moment Closure (CMC) turbulent combustion model have been performed. The aim is to investigate the feasibility of the use of CMC/LES for ignition problems and to examine which, if any, of the characteristics already observed in related experiments could be predicted. A three-dimensional formulation of the CMC equation was used with simple and detailed chemical mechanisms, and sparks with different parameters (location, size) were used. It was found that the correct pattern of flame expansion and overall flame appearance were predicted with reasonable accuracy with both mechanisms, but the detailed mechanism resulted in expansion rates closer to the experiment. Moreover, the distribution of OH was predicted qualitatively accurately, with patches of high and low concentration in the recirculation zone during the ignition transient, consistent with experimental data. The location of the spark relative to the recirculation zone was found to determine the pattern of the flame propagation and the total time for the flame stabilisation. The size was also an important parameter, since it was found that the flame extinguishes when the spark is very small, in agreement with expectations from experiment. The stabilisation mechanism of the flame was dominated by the convection and sub-grid scale diffusion of hot combustion products from the recirculation zone to the cold gases that enter the burner, as revealed by analysis of the CMC equation. (author)

  15. In situ TDLAS measurement of absolute acetylene concentration profiles in a non-premixed laminar counter-flow flame

    NASA Astrophysics Data System (ADS)

    Wagner, S.; Klein, M.; Kathrotia, T.; Riedel, U.; Kissel, T.; Dreizler, A.; Ebert, V.

    2012-06-01

    Acetylene (C2H2), as an important precursor for chemiluminescence species, is a key to understand, simulate and model the chemiluminescence and the related reaction paths. Hence we developed a high resolution spectrometer based on direct Tunable Diode Laser Absorption Spectroscopy (TDLAS) allowing the first quantitative, calibration-free and spatially resolved in situ C2H2 measurement in an atmospheric non-premixed counter-flow flame supported on a Tsuji burner. A fiber-coupled distributed feedback diode laser near 1535 nm was used to measure several absolute C2H2 concentration profiles (peak concentrations up to 9700 ppm) in a laminar non-premixed CH4/air flame ( T up to 1950 K) supported on a modified Tsuji counter-flow burner with N2 purge slots to minimize end flames. We achieve a fractional optical resolution of up to 5×10-5 OD (1 σ) in the flame, resulting in temperature-dependent acetylene detection limits for the P17e line at 6513 cm-1 of up to 2.1 ppmṡm. Absolute C2H2 concentration profiles were obtained by translating the burner through the laser beam using a DC motor with 100 μm step widths. Intercomparisons of the experimental C2H2 profiles with simulations using our new hydrocarbon oxidation mechanisms show excellent agreement in position, shape and in the absolute C2H2 values.

  16. Effect of the composition of the hot product stream in the quasi-steady extinction of strained premixed flames

    SciTech Connect

    Coriton, Bruno; Smooke, Mitchell D.; Gomez, Alessandro

    2010-11-15

    The extinction of premixed CH{sub 4}/O{sub 2}/N{sub 2} flames counterflowing against a jet of combustion products in chemical equilibrium was investigated numerically using detailed chemistry and transport mechanisms. Such a problem is of relevance to combustion systems with non-homogeneous air/fuel mixtures or recirculation of the burnt gases. Contrary to similar studies that were focused on heat loss/gain, depending on the degree of non-adiabaticity of the system, the emphasis here was on the yet unexplored role of the composition of counterflowing burnt gases in the extinction of lean-to-stoichiometric premixed flames. For a given temperature of the counterflowing products of combustion, it was found that the decrease of heat release with increase in strain rate could be either monotonic or non-monotonic, depending on the equivalence ratio {phi}{sub b} of the flame feeding the hot combustion product stream. Two distinct extinction modes were observed: an abrupt one, when the hot counterflowing stream consists of either inert gas or equilibrium products of a stoichiometric premixed flame, and a smooth extinction, when there is an excess of oxidizing species in the combustion product stream. In the latter case four burning regimes can be distinguished as the strain rate is progressively increased while the heat release decreases smoothly: an adiabatic propagating flame regime, a non-adiabatic propagating flame regime, the so-called partially-extinguished flame regime, in which the location of the peak of heat release crosses the stagnation plane, and a frozen flow regime. The flame structure was analyzed in detail in the different burning regimes. Abrupt extinction was attributed to the quenching of the oxidation layer with the entire H-OH-O radical pool being comparably reduced. Under conditions of smooth extinction, the behavior is different and the concentration of the H radical decreases the most with increasing strain rate, whereas OH and O remain

  17. Nitric oxide formation in a lean, premixed-prevaporized jet A/air flame tube: An experimental and analytical study

    NASA Technical Reports Server (NTRS)

    Lee, Chi-Ming; Bianco, Jean; Deur, John M.; Ghorashi, Bahman

    1992-01-01

    An experimental and analytical study was performed on a lean, premixed-prevaporized Jet A/air flame tube. The NO(x) emissions were measured in a flame tube apparatus at inlet temperatures ranging from 755 to 866 K (900 to 1100 F), pressures from 10 to 15 atm, and equivalence ratios from 0.37 to 0.62. The data were then used in regressing an equation to predict the NO(x) production levels in combustors of similar design. Through an evaluation of parameters it was found that NO(x) is dependent on adiabatic flame temperature and combustion residence time, yet independent of pressure and inlet air temperature for the range of conditions studied. This equation was then applied to experimental data that were obtained from the literature, and a good correlation was achieved.

  18. Strain rate and fuel composition dependence of chemiluminescent species profiles in non-premixed counterflow flames: comparison with model results

    NASA Astrophysics Data System (ADS)

    Prabasena, B.; Röder, M.; Kathrotia, T.; Riedel, U.; Dreier, T.; Schulz, C.

    2012-06-01

    A detailed comparison has been conducted between chemiluminescence (CL) species profiles of OH∗, CH∗, and C2 ∗, obtained experimentally and from detailed flame kinetics modeling, respectively, of atmospheric pressure non-premixed flames formed in the forward stagnation region of a fuel flow ejected from a porous cylinder and an air counterflow. Both pure methane and mixtures of methane with hydrogen (between 10 and 30 % by volume) were used as fuels. By varying the air-flow velocities methane flames were operated at strain rates between 100 and 350 s-1, while for methane/hydrogen flames the strain rate was fixed at 200 s-1. Spatial profiles perpendicular to the flame front were extracted from spectrograms recorded with a spectrometer/CCD camera system and evaluating each spectral band individually. Flame kinetics modeling was accomplished with an in-house chemical mechanism including C1-C4 chemistry, as well as elementary steps for the formation, removal, and electronic quenching of all measured active species. In the CH4/air flames, experiments and model results agree with respect to trends in profile peak intensity and position. For the CH4/H2/air flames, with increasing H2 content in the fuel the experimental CL peak intensities decrease slightly and their peak positions shift towards the fuel side, while for the model the drop in mole fraction is much stronger and the peak positions move closer to the fuel side. For both fuel compositions the modeled profiles peak closer to the fuel side than in the experiments. The discrepancies can only partly be attributed to the limited attainable spatial resolution but may also necessitate revised reaction mechanisms for predicting CL species in this type of flame.

  19. A detailed kinetic modeling study of toluene oxidation in a premixed laminar flame

    SciTech Connect

    Tian, Z; Pitz, W J; Fournet, R; Glaude, P; Battin-Leclerc, F

    2009-12-18

    An improved chemical kinetic model for the toluene oxidation based on experimental data obtained in a premixed laminar low-pressure flame with vacuum ultraviolet (VUV) photoionization and molecular beam mass spectrometry (MBMS) techniques has been proposed. The present mechanism consists of 273 species up to chrysene and 1740 reactions. The rate constants of reactions of toluene, decomposition, reaction with oxygen, ipso-additions and metatheses with abstraction of phenylic H-atom are updated; new pathways of C{sub 4} + C{sub 2} species giving benzene and fulvene are added. Based on the experimental observations, combustion intermediates such as fulvenallene, naphtol, methylnaphthalene, acenaphthylene, 2-ethynylnaphthalene, phenanthrene, anthracene, 1-methylphenanthrene, pyrene and chrysene are involved in the present mechanism. The final toluene model leads to an overall satisfactory agreement between the experimentally observed and predicted mole fraction profiles for the major products and most combustion intermediates. The toluene depletion is governed by metathese giving benzyl radicals, ipso-addition forming benzene and metatheses leading to C{sub 6}H{sub 4}CH{sub 3} radicals. A sensitivity analysis indicates that the unimolecular decomposition via the cleavage of a C-H bond has a strong inhibiting effect, while decomposition via C-C bond breaking, ipso-addition of H-atom to toluene, decomposition of benzyl radicals and reactions related to C{sub 6}H{sub 4}CH{sub 3} radicals have promoting effect for the consumption of toluene. Moreover, flow rate analysis is performed to illustrate the formation pathways of mono- and polycyclic aromatics.

  20. Effects of buoyancy on lean premixed v-flames, Part II. VelocityStatistics in Normal and Microgravity

    SciTech Connect

    Cheng, R.K.; Bedat, B.; Yegian, D.T.

    1999-07-01

    The field effects of buoyancy on laminar and turbulent premixed v-flames have been studied by the use of laser Doppler velocimetry to measure the velocity statistics in +1g, -1g and {micro}g flames. The experimental conditions covered mean velocity, Uo, of 0.4 to 2 m/s, methane/air equivalence ratio, f, of 0.62 to 0.75. The Reynolds numbers, from 625 to 3130 and the Richardson number from 0.05 to 1.34. The results show that a change from favorable (+1g) to unfavorable (-1g) mean pressure gradient in the plume create stagnating flows in the far field whose influences on the mean and fluctuating velocities persist in the near field even at the highest Re we have investigated. The use of Richardson number < 0.1 as a criterion for momentum dominance is not sufficient to prescribe an upper limit for these buoyancy effects. In {micro}g, the flows within the plumes are non-accelerating and parallel. Therefore, velocity gradients and hence mean strain rates in the plumes of laboratory flames are direct consequences of buoyancy. Furthermore, the rms fluctuations in the plumes of {micro}g flames are lower and more isotropic than in the laboratory flames to show that the unstable plumes in laboratory flames also induce velocity fluctuations. The phenomena influenced by buoyancy i.e. degree of flame wrinkling, flow acceleration, flow distribution, and turbulence production, can be subtle due to their close coupling with other flame flow interaction processes. But they cannot be ignored in fundamental studies or else the conclusions and insights would be ambiguous and not very meaningful.

  1. Response analysis of a laminar premixed M-flame to flow perturbations using a linearized compressible Navier-Stokes solver

    SciTech Connect

    Blanchard, M.; Schuller, T.; Sipp, D.; Schmid, P. J.

    2015-04-15

    The response of a laminar premixed methane-air flame subjected to flow perturbations around a steady state is examined experimentally and using a linearized compressible Navier-Stokes solver with a one-step chemistry mechanism to describe combustion. The unperturbed flame takes an M-shape stabilized both by a central bluff body and by the external rim of a cylindrical nozzle. This base flow is computed by a nonlinear direct simulation of the steady reacting flow, and the flame topology is shown to qualitatively correspond to experiments conducted under comparable conditions. The flame is then subjected to acoustic disturbances produced at different locations in the numerical domain, and its response is examined using the linearized solver. This linear numerical model then allows the componentwise investigation of the effects of flow disturbances on unsteady combustion and the feedback from the flame on the unsteady flow field. It is shown that a wrinkled reaction layer produces hydrodynamic disturbances in the fresh reactant flow field that superimpose on the acoustic field. This phenomenon, observed in several experiments, is fully interpreted here. The additional perturbations convected by the mean flow stem from the feedback of the perturbed flame sheet dynamics onto the flow field by a mechanism similar to that of a perturbed vortex sheet. The different regimes where this mechanism prevails are investigated by examining the phase and group velocities of flow disturbances along an axis oriented along the main direction of the flow in the fresh reactant flow field. It is shown that this mechanism dominates the low-frequency response of the wrinkled shape taken by the flame and, in particular, that it fully determines the dynamics of the flame tip from where the bulk of noise is radiated.

  2. Effects of Turbulence on the Combustion Properties of Partially Premixed Flames of Canola Methyl Ester and Diesel Blends

    DOE PAGESBeta

    Dhamale, N.; Parthasarathy, R. N.; Gollahalli, S. R.

    2011-01-01

    Canola methyl ester (CME) is a biofuel that is a renewable alternative energy resource and is produced by the transesterification of canola oil. The objective of this study was to document the effects of turbulence on the combustion characteristics of blends of CME and No 2 diesel fuel in a partially-premixed flame environment. The experiments were conducted with mixtures of pre-vaporized fuel and air at an initial equivalence ratio of 7 and three burner exit Reynolds numbers, 2700, 3600, and 4500. Three blends with 25, 50, and 75% volume concentration of CME were studied. The soot volume fraction was highestmore » for the pure diesel flames and did not change significantly with Reynolds number due to the mutually compensating effects of increased carbon input rate and increased air entrainment as the Reynolds number was increased. The global NOx emission index was highest and the CO emission index was the lowest for the pure CME flame, and varied non-monotonically with biofuel content in the blend The mean temperature and the NOx concentration at three-quarter flame height were generally correlated, indicating that the thermal mechanism of NOx formation was dominant in the turbulent biofuel flames also.« less

  3. Two-time correlation of heat release rate and spectrum of combustion noise from turbulent premixed flames

    NASA Astrophysics Data System (ADS)

    Liu, Yu

    2015-09-01

    The spectral characteristics of combustion noise are dictated by the temporal correlation of the overall change of heat release rate fluctuations which has not received sufficient attention in prior studies. In this work, the two-time correlation of the volumetric heat release rate fluctuations within the flame brush and its role in modeling combustion noise spectrum are investigated by analyzing direct numerical simulation (DNS) data of turbulent premixed V-flames. This two-time correlation can be well represented by Gaussian-type functions and it captures the slow global variation of the fluctuating heat release rate and hence the low-frequency noise sources of unsteady combustion. The resulting correlation model is applied to predict the far-field noise spectrum from test open flames, and different reference time scales are used to scale this correlation from the DNS data to the test flames. The comparison between predictions and measurements indicates that the correlation models of all reference time scales are capable of reproducing the essential spectral shape including the low- and high-frequency dependencies. Reasonable agreement in the peak frequency, peak sound pressure level, and the Strouhal number scaling of peak frequency is also achieved for two turbulent time scales. A promising convective time scale shows great potential for characterizing the spectral features, yet its predictive capabilities are to be further verified through a longer DNS signal of a bounded flame configuration.

  4. High-speed laser diagnostics for the study of flame dynamics in a lean premixed gas turbine model combustor

    NASA Astrophysics Data System (ADS)

    Boxx, Isaac; Arndt, Christoph M.; Carter, Campbell D.; Meier, Wolfgang

    2012-03-01

    A series of measurements was taken on two technically premixed, swirl-stabilized methane-air flames (at overall equivalence ratios of ϕ = 0.73 and 0.83) in an optically accessible gas turbine model combustor. The primary diagnostics used were combined planar laser-induced fluorescence of the OH radical and stereoscopic particle image velocimetry (PIV) with simultaneous repetition rates of 10 kHz and a measurement duration of 0.8 s. Also measured were acoustic pulsations and OH chemiluminescence. Analysis revealed strong local periodicity in the thermoacoustically self-excited (or ` noisy') flame (ϕ = 0.73) in the regions of the flow corresponding to the inner shear layer and the jet-inflow. This periodicity appears to be the result of a helical precessing vortex core (PVC) present in that region of the combustor. The PVC has a precession frequency double (at 570 Hz) that of the thermo-acoustic pulsation (at 288 Hz). A comparison of the various data sets and analysis techniques applied to each flame suggests a strong coupling between the PVC and the thermo-acoustic pulsation in the noisy flame. Measurements of the stable (` quiet') flame (ϕ = 0.83) revealed a global fluctuation in both velocity and heat-release around 364 Hz, but no clear evidence of a PVC.

  5. Experimental Characterization of Combustion Instabilities and Flow-Flame Dynamics in a Partially-Premixed Gas Turbine Model Combustor

    NASA Astrophysics Data System (ADS)

    Allison, Patton Manuel

    Partially-premixed, swirl combustion is applied in gas turbine combustors to achieve flame stabilization and reduced emission production. However, this method is also inherently sensitive to combustion instabilities which can cause large pressure, velocity, and heat release fluctuations. This thesis investigates thermoacoustic coupling created by flow-flame dynamics in a gas turbine model combustor (GTMC) for a variety of fuels and operating flow rates. Several naturally occurring instability modes were identified to control the acoustic response of the system, including Helmholtz resonances from the plenum and convective-acoustic effects which cause equivalence ratio oscillations. Laser Doppler velocimetry was used to measure radial flow in the GTMC, which can set up flow-fields which create loudly resonating flat-shaped flames, in comparison to quiet V-shaped flames. Flame location and shape altered convective time delays which determine the relative phases of pressure and heat release oscillations. Simultaneous pressure and chemiluminescence imaging showed that the heat release, pressure fluctuations, and flame motion are all coupled at the same instability frequency. Videos of the flame motion also revealed that the precessing vortex core (PVC), created by the swirling flow, influences the rocking behavior of the flame. Acetone was added to the fuel to act as a tracer in fluorescence measurements which indicated the localization of unburned fuel. It was discovered that fuel was distributed in lobes which corresponded to locations surrounding the shear layer outside of the central recirculation zone, and that the relative distribution of the lobes adjusted to forcing by the flow. Finally, high-speed formaldehyde planar laser-induced fluorescence was applied to study the motion of preheat zone surfaces in response to the oscillations of the instability. The flame surface density and wrinkling fluctuated at the acoustic frequency and displayed dampened motions

  6. Transient change in the shape of premixed burner flame with the superposition of pulsed dielectric barrier discharge

    NASA Astrophysics Data System (ADS)

    Zaima, Kazunori; Sasaki, Koichi

    2016-08-01

    We investigated the transient phenomena in a premixed burner flame with the superposition of a pulsed dielectric barrier discharge (DBD). The length of the flame was shortened by the superposition of DBD, indicating the activation of combustion chemical reactions with the help of the plasma. In addition, we observed the modulation of the top position of the unburned gas region and the formations of local minimums in the axial distribution of the optical emission intensity of OH. These experimental results reveal the oscillation of the rates of combustion chemical reactions as a response to the activation by pulsed DBD. The cycle of the oscillation was 0.18–0.2 ms, which could be understood as the eigenfrequency of the plasma-assisted combustion reaction system.

  7. Transient change in the shape of premixed burner flame with the superposition of pulsed dielectric barrier discharge

    NASA Astrophysics Data System (ADS)

    Zaima, Kazunori; Sasaki, Koichi

    2016-08-01

    We investigated the transient phenomena in a premixed burner flame with the superposition of a pulsed dielectric barrier discharge (DBD). The length of the flame was shortened by the superposition of DBD, indicating the activation of combustion chemical reactions with the help of the plasma. In addition, we observed the modulation of the top position of the unburned gas region and the formations of local minimums in the axial distribution of the optical emission intensity of OH. These experimental results reveal the oscillation of the rates of combustion chemical reactions as a response to the activation by pulsed DBD. The cycle of the oscillation was 0.18-0.2 ms, which could be understood as the eigenfrequency of the plasma-assisted combustion reaction system.

  8. A Detailed Chemical Kinetic Reaction Mechanism for Oxidation of Four Small Alkyl Esters in Laminar Premixed Flames

    SciTech Connect

    Westbrook, C K; Pitz, W J; Westmoreland, P R; Dryer, F L; Chaos, M; Osswald, P; Kohse-Hoinghaus, K; Cool, T A; Wang, J; Yang, B; Hansen, N; Kasper, T

    2008-02-08

    A detailed chemical kinetic reaction mechanism has been developed for a group of four small alkyl ester fuels, consisting of methyl formate, methyl acetate, ethyl formate and ethyl acetate. This mechanism is validated by comparisons between computed results and recently measured intermediate species mole fractions in fuel-rich, low pressure, premixed laminar flames. The model development employs a principle of similarity of functional groups in constraining the H atom abstraction and unimolecular decomposition reactions in each of these fuels. As a result, the reaction mechanism and formalism for mechanism development are suitable for extension to larger oxygenated hydrocarbon fuels, together with an improved kinetic understanding of the structure and chemical kinetics of alkyl ester fuels that can be extended to biodiesel fuels. Variations in concentrations of intermediate species levels in these flames are traced to differences in the molecular structure of the fuel molecules.

  9. Characterization of temperature non-uniformity over a premixed CH4-air flame based on line-of-sight TDLAS

    NASA Astrophysics Data System (ADS)

    Zhang, Guangle; Liu, Jianguo; Xu, Zhenyu; He, Yabai; Kan, Ruifeng

    2016-01-01

    A novel technique for characterizing temperature non-uniformity has been investigated based on measurements of line-of-sight tunable diode laser absorption spectroscopy. It utilized two fiber-coupled distributed feedback diode lasers at wavelengths around 1339 and 1392 nm as light sources to probe the field at multiple absorptions lines of water vapor and applied a temperature binning strategy combined with Gauss-Seidel iteration method to explore the temperature non-uniformity of the field in one dimension. The technique has been applied to a McKenna burner, which produced a flat premixed laminar CH4-air flame. The flame and its adjacent area formed an atmospheric field with significant non-uniformity of temperature and water vapor concentration. The effect of the number of temperature bins on column-density and temperature results has also been explored.

  10. Propagation and extinction of premixed C{sub 5}-C{sub 12}n-alkane flames

    SciTech Connect

    Ji, Chunsheng; Dames, Enoch; Wang, Yang L.; Wang, Hai; Egolfopoulos, Fokion N.

    2010-02-15

    Laminar flame speeds and extinction strain rates of premixed C{sub 5}-C{sub 12}n-alkane flames were determined at atmospheric pressure and elevated unburned mixture temperatures, over a wide range of equivalence ratios. Experiments were performed in the counterflow configuration and flow velocities were measured using Laser Doppler Velocimetry. The laminar flame speeds were obtained using a non-linear extrapolation technique utilizing numerical simulations of the counterflow experiments with detailed descriptions of chemical kinetics and molecular transport. Compared to linearly extrapolated values, the laminar flame speeds obtained using non-linear extrapolations were found to be 1-4 cm/s lower depending on the equivalence ratio. It was determined that the laminar flame speeds of all n-alkane/air mixtures considered in this investigation are similar to each other and sensitive largely to the H{sub 2}/CO and C{sub 1}-C{sub 4} hydrocarbon kinetics. Additionally, the resistance to extinction decreases as the fuel molecular weight increases. Simulations of the experiments were performed using the recently developed JetSurF 0.2 reaction model consisting of 194 species and 1459 reactions. The laminar flame speeds were predicted with good accuracy for all the n-alkane-air mixtures considered. The experimental extinction strain rates are well predicted by the model for fuel-lean mixtures. For stoichiometric and fuel-rich mixtures, the predicted extinction strain rates are approximately 10% lower than the experimental values. Insights into the physical and chemical processes that control the response of n-alkane flames are provided through detailed sensitivity analyses on both reaction rates and binary diffusion coefficients. (author)

  11. Application of the conditional source-term estimation model for turbulence-chemistry interactions in a premixed flame

    NASA Astrophysics Data System (ADS)

    Salehi, M. M.; Bushe, W. K.; Daun, K. J.

    2012-04-01

    Conditional Source-term Estimation (CSE) is a closure model for turbulence-chemistry interactions. This model uses the first-order CMC hypothesis to close the chemical reaction source terms. The conditional scalar field is estimated by solving an integral equation using inverse methods. It was originally developed and has been used extensively in non-premixed combustion. This work is the first application of this combustion model for a premixed flame. CSE is coupled with a Trajectory Generated Low-Dimensional Manifold (TGLDM) model for chemistry. The CSE-TGLDM combustion model is used in a RANS code to simulate a turbulent premixed Bunsen burner. Along with this combustion model, a similar model which relies on the flamelet assumption is also used for comparison. The results of these two approaches in the prediction of the velocity field, temperature and species mass fractions are compared together. Although the flamelet model is less computationally expensive, the CSE combustion model is more general and does not have the limiting assumption underlying the flamelet model.

  12. TIME-VARYING FLAME IONIZATION SENSING APPLIED TO NATURAL GAS AND PROPANE BLENDS IN A PRESSURIZED LEAN PREMIXED (LPM) COMBUSTOR

    SciTech Connect

    D. L. Straub; B. T. Chorpening; E. D. Huckaby; J. D. Thornton; W. L. Fincham

    2008-06-13

    In-situ monitoring of combustion phenomena is a critical need for optimal operation and control of advanced gas turbine combustion systems. The concept described in this paper is based on naturally occurring flame ionization processes that accompany the combustion of hydrocarbon fuels. Previous work has shown that flame ionization techniques may be applied to detect flashback, lean blowout, and some aspects of thermo-acoustic combustion instabilities. Previous work has focused on application of DC electric fields. By application of time-varying electric fields, significant improvements to sensor capabilities have been observed. These data have been collected in a lean premixed combustion test rig operating at 0.51-0.76 MPa (5-7.5 atm) with air preheated to 588 K (600°F). Five percent of the total fuel flow is injected through the centerbody tip as a diffusion pilot. The fuel composition is varied independently by blending approximately 5% (volume) propane with the pipeline natural gas. The reference velocity through the premixing annulus is kept constant for all conditions at a nominal value of 70 m/s. The fuel-air equivalence ratio is varied independently from 0.46 – 0.58. Relative to the DC field version, the time-varying combustion control and diagnostic sensor (TV-CCADS) shows a significant improvement in the correlation between the measured flame ionization current and local fuel-air equivalence ratio. In testing with different fuel compositions, the triangle wave data show the most distinct change in flame ionization current in response to an increase in propane content. Continued development of this sensor technology will improve the capability to control advanced gas turbine combustion systems, and help address issues associated with variations in fuel supplies.

  13. Flame behaviors of propane/air premixed flame propagation in a closed rectangular duct with a 90-deg bend

    NASA Astrophysics Data System (ADS)

    He, Xuechao; Sun, Jinhua; Yuen, K. K.; Ding, Yibin; Chen, Sining

    2008-11-01

    Experiments of flame propagation in a small, closed rectangular duct with a 90° bend were performed for a propane-air mixture. The high speed camera and Schlieren techniques were used to record images of flame propagation process in the combustion pipe. Meanwhile, the fine thermocouples and ion current probes were applied to measure the temperature distribution and reaction intensity of combustion. The characteristics of propane-air flame and its microstructure were analyzed in detail by the experimental results. In the test, the special tulip flame formation was observed. Around the bend, the flame tip proceeded more quickly at the lower side with the flame front elongated toward the axial direction. And transition to turbulent flame occurred. It was suggested that fluctuations of velocity, ion current and temperature were mainly due to the comprehensive effects of multi-wave and the intense of turbulent combustion.

  14. An experimental study of low-pressure premixed pyrrole/oxygen/argon flames with tunable synchrotron photoionization

    SciTech Connect

    Tian, Zhenyu; Li, Yuyang; Zhang, Taichang; Qi, Fei; Zhu, Aiguo; Cui, Zhifeng

    2007-10-15

    Two premixed laminar pyrrole/oxygen/argon flames at 3.33 kPa (25 Torr) with equivalence ratios of 0.55 (C/O/N = 1:5.19:0.25) and 1.84 (C/O/N = 1:1.56:0.25) have been investigated using tunable synchrotron photoionization and molecular-beam mass spectrometry techniques. All observed flame species, including some nitrogen-containing intermediates, have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of species including reactants, intermediates, and products have been determined by scanning burner position at some selected photon energies near ionization thresholds, and flame temperature has been measured by a Pt/Pt-13% Rh thermocouple. The results indicate that N{sub 2}, NO, and NO{sub 2} are the major nitrogenous products, while hydrogen cyanide, isocyanic acid, and 2-propenenitrile are the most important nitrogen-containing intermediates in pyrrole flames. Radicals such as methyl, propargyl, allyl, cyanomethyl, n-propyl, isobutyl, cyclopentadienyl, phenyl, cyclohexyl, phenoxy, and 4-methylbenzyl are observed as well. Moreover, ethenol and methylacrylonitrile are also detected. Reaction pathways involving the major species are proposed. The new results will be useful in developing a kinetic model of nitrogenous compound combustion. (author)

  15. Diode laser absorption measurement and analysis of HCN in atmospheric-pressure, fuel-rich premixed methane/air flames

    SciTech Connect

    Gersen, S.; Mokhov, A.V.; Levinsky, H.B.

    2008-10-15

    Measurements of HCN in flat, fuel-rich premixed methane/air flames at atmospheric pressure are reported. Quartz-microprobe sampling followed by wavelength modulation absorption spectroscopy with second harmonic detection was used to obtain an overall measurement uncertainty of better than 20% for mole fractions HCN on the order of 10 ppm. The equivalence ratio, {phi}, was varied between 1.3 and 1.5, while the flame temperature was varied independently by changing the mass flux through the burner surface at constant equivalence ratio. Under the conditions of the experiments, the peak mole fractions vary little, in the range of 10-15 ppm. Increasing the flame temperature by increasing the mass flux had little influence on the peak mole fraction, but accelerated HCN burnout substantially. At high equivalence ratio and low flame temperature, HCN burnout is very slow: at {phi}=1.5, {proportional_to}10ppm HCN is still present 7 mm above the burner surface. Substantial quantitative disagreement is observed between the experimental profiles and those obtained from calculations using GRI-Mech 3.0, with the calculations generally overpredicting the results significantly. Changing the rates of key formation and consumption reactions for HCN can improve the agreement, but only by making unreasonable changes in these rates. Inclusion of reactions describing NCN formation and consumption in the calculations improves the agreement with the measurements considerably. (author)

  16. Dimensionality estimate of the manifold in chemical composition space for a turbulent premixed H2+air flame

    SciTech Connect

    Tonse, Shaheen R.; Brown, Nancy J.

    2003-02-26

    The dimensionality (D) of manifolds of active chemical composition space has been measured using three different approaches: the Hausdorff geometrical binning method, Principal Component Analysis, and the Grassberger-Procaccia cumulative distribution method. A series of artificial manifolds is also generated using a Monte Carlo approach to discern the advantages and limitations of the three methods. Dimensionality is quantified for different levels of turbulent intensity in a simulation of the interactions of a 2D premixed hydrogen flame with a localized region of turbulence superimposed over the cold region upstream of the flame front. The simulations are conducted using an adaptive mesh refinement code for low Mach number reacting flows. By treating the N{sub s} species and temperature of the local thermo-chemical state as a point in multi-dimensional chemical composition space, a snapshot of a flame region is mapped into chemical composition space to generate the manifold associated with the 2-D flame system. An increase in D was observed with increasing turbulent intensity for all three methods. Although each method provides useful information, the Grassberger-Procaccia method is subject to fewer artifacts than the other two thereby providing the most reliable quantification of D.

  17. Experimental study of vorticity-strain rate interaction in turbulent partially-premixed jet flames using tomographic particle image velocimetry

    DOE PAGESBeta

    Coriton, Bruno; Frank, Jonathan H.

    2016-02-16

    In turbulent flows, the interaction between vorticity, ω, and strain rate, s, is considered a primary mechanism for the transfer of energy from large to small scales through vortex stretching. The ω-s coupling in turbulent jet flames is investigated using tomographic particle image velocimetry (TPIV). TPIV provides a direct measurement of the three-dimensional velocity field from which ω and s are determined. The effects of combustion and mean shear on the ω-s interaction are investigated in turbulent partially premixed methane/air jet flames with high and low probabilities of localized extinction as well as in a non-reacting isothermal air jet withmore » Reynolds number of approximately 13,000. Results show that combustion causes structures of high vorticity and strain rate to agglomerate in highly correlated, elongated layers that span the height of the probe volume. In the non-reacting jet, these structures have a more varied morphology, greater fragmentation, and are not as well correlated. The enhanced spatiotemporal correlation of vorticity and strain rate in the stable flame results in stronger ω-s interaction characterized by increased enstrophy and strain-rate production rates via vortex stretching and straining, respectively. The probability of preferential local alignment between ω and the eigenvector of the intermediate principal strain rate, s2, which is intrinsic to the ω-s coupling in turbulent flows, is larger in the flames and increases with the flame stability. The larger mean shear in the flame imposes a preferential orientation of ω and s2 tangential to the shear layer. The extensive and compressive principal strain rates, s1 and s3, respectively, are preferentially oriented at approximately 45° with respect to the jet axis. As a result, the production rates of strain and vorticity tend to be dominated by instances in which ω is parallel to the s1¯-s2¯ plane and orthogonal to s3¯.« less

  18. Investigation of non-premixed flame combustion characters in GO2/GH2 shear coaxial injectors using non-intrusive optical diagnostics

    NASA Astrophysics Data System (ADS)

    Dai, Jian; Yu, NanJia; Cai, GuoBiao

    2015-12-01

    Single-element combustor experiments are conducted for three shear coaxial geometry configuration injectors by using gaseous oxygen and gaseous hydrogen (GO2/GH2) as propellants. During the combustion process, several spatially and timeresolved non-intrusive optical techniques, such as OH planar laser induced fluorescence (PLIF), high speed imaging, and infrared imaging, are simultaneously employed to observe the OH radical concentration distribution, flame fluctuations, and temperature fields. The results demonstrate that the turbulent flow phenomenon of non-premixed flame exhibits a remarkable periodicity, and the mixing ratio becomes a crucial factor to influence the combustion flame length. The high speed and infrared images have a consistent temperature field trend. As for the OH-PLIF images, an intuitionistic local flame structure is revealed by single-shot instantaneous images. Furthermore, the means and standard deviations of OH radical intensity are acquired to provide statistical information regarding the flame, which may be helpful for validation of numerical simulations in future. Parameters of structure configurations, such as impinging angle and oxygen post thickness, play an important role in the reaction zone distribution. Based on a successful flame contour extraction method assembled with non-linear anisotropic diffusive filtering and variational level-set, it is possible to implement a fractal analysis to describe the fractal characteristics of the non-premixed flame contour. As a result, the flame front cannot be regarded as a fractal object. However, this turbulent process presents a self-similarity characteristic.

  19. Local consumption speed of turbulent premixed flames - An analysis of ''memory effects''

    SciTech Connect

    Hemchandra, Santosh; Lieuwen, Tim

    2010-05-15

    The local turbulent flame speed of an attached flame is not only a function of the local flow and flame conditions, but also of upstream conditions - i.e., it is ''non-local'' or exhibits ''memory''. Non-locality adds an additional degree of freedom to the classic problem of a freely propagating flame propagating normally to the time averaged flow. Non-locality occurs due to mean tangential flow along the flame brush, which causes flame wrinkles to translate downstream. As such, the wrinkling of the flame at any given point is not only a function of the local velocity disturbance, but also a superposition of flame surface perturbations from locations upstream at previous times. This causes the correlation length scale of turbulent flame wrinkles to differ from that of the underlying turbulent velocity fluctuations. The objective of this paper is to provide a physical description of the key flame kinematic processes that cause these non-local effects. Two approaches are adopted in this work. First, analytical solutions of the G-equation that explicitly describe the effect of non-locality in the low turbulence limit are developed. Second, numerical computations of the G-equation are performed that demonstrate the role of non-linearity in flame surface kinematics at higher turbulence intensities. Finally, these predictions are shown to be consistent with data from a turbulent Bunsen flame. (author)

  20. Chemical structures of low-pressure premixed methylcyclohexane flames as benchmarks for the development of a predictive combustion chemistry model

    SciTech Connect

    Skeen, Scott A.; Yang, Bin; Jasper, Ahren W.; Pitz, William J.; Hansen, Nils

    2011-11-14

    The chemical compositions of three low-pressure premixed flames of methylcyclohexane (MCH) are investigated with the emphasis on the chemistry of MCH decomposition and the formation of aromatic species, including benzene and toluene. The flames are stabilized on a flat-flame (McKenna type) burner at equivalence ratios of φ = 1.0, 1.75, and 1.9 and at low pressures between 15 Torr (= 20 mbar) and 30 Torr (= 40 mbar). The complex chemistry of MCH consumption is illustrated in the experimental identification of several C7H12, C7H10, C6H12, and C6H10 isomers sampled from the flames as a function of distance from the burner. Three initiation steps for MCH consumption are discussed: ring-opening to heptenes and methyl-hexenes (isomerization), methyl radical loss yielding the cyclohexyl radical (dissociation), and H abstraction from MCH. Mole fraction profiles as a function of distance from the burner for the C7 species supplemented by theoretical calculations are presented, indicating that flame structures resulting in steeper temperature gradients and/or greater peak temperatures can lead to a relative increase in MCH consumption through the dissociation and isomerization channels. Trends observed among the stable C6 species as well as 1,3-pentadiene and isoprene also support this conclusion. Relatively large amounts of toluene and benzene are observed in the experiments, illustrating the importance of sequential H-abstraction steps from MCH to toluene and from cyclohexyl to benzene. Furthermore, modeled results using the detailed chemical model of Pitz et al. (Proc. Combust. Inst.2007, 31, 267–275) are also provided to illustrate the use of these data as a benchmark for the improvement or future development of a MCH mechanism.

  1. Chemical structures of low-pressure premixed methylcyclohexane flames as benchmarks for the development of a predictive combustion chemistry model

    DOE PAGESBeta

    Skeen, Scott A.; Yang, Bin; Jasper, Ahren W.; Pitz, William J.; Hansen, Nils

    2011-11-14

    The chemical compositions of three low-pressure premixed flames of methylcyclohexane (MCH) are investigated with the emphasis on the chemistry of MCH decomposition and the formation of aromatic species, including benzene and toluene. The flames are stabilized on a flat-flame (McKenna type) burner at equivalence ratios of φ = 1.0, 1.75, and 1.9 and at low pressures between 15 Torr (= 20 mbar) and 30 Torr (= 40 mbar). The complex chemistry of MCH consumption is illustrated in the experimental identification of several C7H12, C7H10, C6H12, and C6H10 isomers sampled from the flames as a function of distance from the burner.more » Three initiation steps for MCH consumption are discussed: ring-opening to heptenes and methyl-hexenes (isomerization), methyl radical loss yielding the cyclohexyl radical (dissociation), and H abstraction from MCH. Mole fraction profiles as a function of distance from the burner for the C7 species supplemented by theoretical calculations are presented, indicating that flame structures resulting in steeper temperature gradients and/or greater peak temperatures can lead to a relative increase in MCH consumption through the dissociation and isomerization channels. Trends observed among the stable C6 species as well as 1,3-pentadiene and isoprene also support this conclusion. Relatively large amounts of toluene and benzene are observed in the experiments, illustrating the importance of sequential H-abstraction steps from MCH to toluene and from cyclohexyl to benzene. Furthermore, modeled results using the detailed chemical model of Pitz et al. (Proc. Combust. Inst.2007, 31, 267–275) are also provided to illustrate the use of these data as a benchmark for the improvement or future development of a MCH mechanism.« less

  2. NO formation in the burnout region of a partially premixed methane-air flame with upstream heat loss

    SciTech Connect

    Mokhov, A.V.; Levinsky, H.B.

    1999-09-01

    Measurements of temperature and NO concentration in laminar, partially premixed methane-air flames stabilized on a ceramic burner in coflow are reported. The NO concentration and temperature were determined by laser-induced fluorescence (LIF) and coherent anti-Stokes Raman scattering (CARS), respectively. Upstream heat loss to the burner was varied by changing the exit velocity of the fuel-air mixture at a constant equivalence ratio of 1,3; this alters the structure of the flame from an axisymmetric Bunsen-type to a strongly stabilized flat flame. To facilitate analysis of the results, a method is derived for separating the effects of dilution from those of chemical reaction based on the relation between the measured temperature and the local mixture fraction, including the effects of upstream heat loss. Using this method, the amount of NO formed during burnout of the hot, fuel-rich combustion products can be ascertained. In the Bunsen-type flame, it is seen that {approximately}40 ppm of NO are produced in this burnout region, at temperatures between {approximately}2,100 K and {approximately}1,900 K, probably via the Zeldovich mechanism. Reducing the exit velocity of 12 cm/s reduces the flame temperature substantially, and effectively eliminates this contribution. At velocities of 12 and 8 cm/s, {approximately}10 ppm of NO are formed in the burnout region, even though the gas temperatures are too low for Zeldovich NO to be significant. Although the mechanism responsible for these observations is as yet unclear, the results are consistent with the idea that the low temperatures in the fuel-rich gases caused by upstream heat loss retard the conversion of HCN (formed via the Fenimore mechanism) to NO, with this residual HCN then being converted to NO during burnout.

  3. Exhaust emissions from a premixing, prevaporizing flame tube using liquid jet A fuel

    NASA Technical Reports Server (NTRS)

    Marek, C. J.; Papathakos, L. C.

    1976-01-01

    Emissions of nitrogen oxides, carbon monoxide, and unburned hydrocarbons were measured in a burner where liquid Jet A fuel was sprayed into the heated air stream and vaporized upstream of a perforated plate flameholder. The burner was tested at inlet air temperatures at 640, 800, and 833 K, an inlet pressure of 5.6 X 100,000 N/m squared, a reference velocity of 25 m/sec, and equivalence ratios from lean blowout to 0.7. Nitrogen oxide levels of below 1.0 g NO2/kg fuel were obtained at combustion efficiencies greater than 99 percent. The measured emission levels for the liquid fuel agreed well with previously reported premixed gaseous propane data and agreed with well stirred reactor predictions. Autoignition of the premixed fuel air mixture was a problem at inlet temperatures above 650 K with 104 msec premixing time.

  4. Effects of platinum stagnation surface on the lean extinction limits of premixed methane/air flames at moderate surface temperatures

    SciTech Connect

    Wiswall, J.T.; Li, J.; Wooldridge, M.S.; Im, H.G.

    2011-01-15

    A stagnation flow reactor was used to study the effects of platinum on the lean flammability limits of atmospheric pressure premixed methane/air flames at moderate stagnation surface temperatures. Experimental and computational methods were used to quantify the equivalence ratio at the lean extinction limit ({phi}{sub ext}) and the corresponding stagnation surface temperature (T{sub s}). A range of flow rates (57-90 cm/s) and corresponding strain rates were considered. The results indicate that the gas-phase methane/air flames are sufficiently strong relative to the heterogeneous chemistry for T{sub s} conditions less than 750 K that the platinum does not affect {phi}{sub ext}. The computational results are in good agreement with the experimentally observed trends and further indicate that higher reactant flow rates (>139 cm/s) and levels of dilution (>{proportional_to}10% N{sub 2}) are required to weaken the gas-phase flame sufficiently for surface reaction to play a positive role on extending the lean flammability limits. (author)

  5. A new apparatus for study of pressure-dependent laminar premixed flames with vacuum ultraviolet photoionization mass spectrometry

    NASA Astrophysics Data System (ADS)

    Zhou, Z. Y.; Wang, Y.; Tang, X. F.; Wu, W. H.; Qi, F.

    2013-01-01

    We report a home-made combustion apparatus for study of pressure-dependent laminar premixed flames with tunable vacuum ultraviolet photoionization mass spectrometry. The instrument consists of a flame chamber, a photoionization chamber with a single-stage sampling system, an ion transfer/storage system, and an orthogonal-acceleration reflectron time-of-flight mass spectrometer. Preliminary results of fuel-rich C2H4/O2/Ar flames at pressures of 30, 150, and 760 Torr have been obtained with this instrument. Compared to previous instruments [T. A. Cool, A. McIlroy, F. Qi, P. R. Westmoreland, L. Poisson, D. S. Peterka, and M. Ahmed, Rev. Sci. Instrum. 76, 094102 (2005), 10.1063/1.2010307; F. Qi, R. Yang, B. Yang, C. Q. Huang, L. X. Wei, J. Wang, L. S. Sheng, and Y. W. Zhang, Rev. Sci. Instrum. 77, 084101 (2006)], 10.1063/1.2234855, performances of the new apparatus have higher mass resolution (˜3500 at m/z = 40), better detection limit (<1 ppm), and broader dynamic range (better than 5 order of magnitude).

  6. Large-eddy simulation/PDF modeling of a non-premixed CO/H2 temporally evolving jet flame

    NASA Astrophysics Data System (ADS)

    Yang, Yue; Wang, Haifeng; Pope, Stephen B.; Chen, Jacqueline H.

    2011-11-01

    We report a large-eddy simulation (LES)/probability density function (PDF) study of a non-premixed CO/H2 temporally evolving planar jet flame at Re = 9079 and Da = 0.011 with skeletal chemistry. The flame exhibits strong turbulence- chemistry interactions resulting in local extinction followed by re-ignition. In this study, the filtered velocity field in LES is computed using the NGA code (Desjardins et al., 2008) and the PDF transported equations with the modified Curl's mixing model are solved by the new highly-scalable HPDF code (Wang and Pope, 2011) with second order accuracy in space and time. The performance of the hybrid LES/PDF methodology is assessed through detailed a posteriori comparisons with DNS of the same flame (Hawkes et al., 2007). The comparison shows good agreement of the temporal evolution of the temperature and mass fractions of major chemical species, as well as the prediction of local extinction and re-ignition. In addition, the effects of the subgrid scale model, the mixing model, and grid resolution on turbulence-chemistry interactions are investigated to improve the capabilities of LES/PDF. Supported in part by the CEFRC funded by the DOE.

  7. Dynamic light scattering in sooting premixed atmospheric-pressure methane-, propane-, ethene-, and propene-oxygen flames

    SciTech Connect

    Lamprecht, A.; Eimer, W.; Kohse-Hoeinghaus, K.

    1999-07-01

    In a systematic investigation under well-defined flame conditions, dynamic light scattering (DLS) was applied to the determination of soot particle radii with the aim of examining the suitability of this technique for accurate soot particle sizing. In particular, flat premixed methane-, propane-, ethene-, and propene-oxygen flames at atmospheric pressure were investigated, and particle sizes were obtained as a function of stoichiometry and height above the burner surface. In combination with absorption measurements, soot volume fraction and particle number density were determined; also, the temperature was measured at each flame condition. In comparison to absorption techniques, attractive features of DLS are its independence of the particle refractive index and its insensitivity to fluorescence interference; also, it offers spatial resolution. In principle, additional information on the particle size distribution as well as on the global shape of the particles may be obtained from DLS experiments. This study is therefore an evaluation of the potential of DLS as a complement to other soot diagnostic techniques.

  8. High-Speed Tomographic PIV Measurements of Strain Rate Properties in Turbulent Partially-Premixed Jet Flames

    NASA Astrophysics Data System (ADS)

    Coriton, Bruno; Frank, Jonathan H.

    2014-11-01

    The effects of combustion on the strain rate field in turbulent jets were studied using 10 kHz tomographic particle image velocimetry (TPIV). Measurements were performed in a series of turbulent partially-premixed jet flames with increasing jet Reynolds numbers and increasing probabilities of localized extinction. Properties of the strain rate were analyzed including the relative ratios of principal strain rates, the preferential alignment of the principal strain rates with vorticity, and the strain rate clustering and intermittency. Comparisons with measurements in turbulent air jets revealed the effects of heat release on the structure and dynamics of the strain rate field. This material is based upon work supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences.

  9. AROMATIC AND POLYCYCLIC AROMATIC HYDROCARBON FORMATION IN A LAMINAR PREMIXED N-BUTANE FLAME. (R825412)

    EPA Science Inventory

    Abstract

    Experimental and detailed chemical kinetic modeling work has been performed to investigate aromatic and polycyclic aromatic hydrocarbon (PAH) formation pathways in a premixed, rich, sooting, n-butane¯oxygen¯argon burner s...

  10. Quantitative measurement of soot particle size distribution in premixed flames - The burner-stabilized stagnation flame approach

    SciTech Connect

    Abid, Aamir D.; Camacho, Joaquin; Sheen, David A.; Wang, Hai

    2009-10-15

    A burner-stabilized, stagnation flame technique is introduced. In this technique, a previously developed sampling probe is combined with a water-cooled circular plate such that the combination simultaneously acts as a flow stagnation surface and soot sample probe for mobility particle sizing. The technique allows for a rigorous definition of the boundary conditions of the flame with probe intrusion and enables less ambiguous comparison between experiment and model. Tests on a 16.3% ethylene-23.7% oxygen-argon flame at atmospheric pressure show that with the boundary temperatures of the burner and stagnation surfaces accurately determined, the entire temperature field may be reproduced by pseudo one-dimensional stagnation reacting flow simulation using these temperature values as the input boundary conditions. Soot particle size distribution functions were determined for the burner-stabilized, stagnation flame at several burner-to-stagnation surface separations. It was found that the tubular probe developed earlier perturbs the flow and flame temperature in a way which is better described by a one-dimensional stagnation reacting flow than by a burner-stabilized flame free of probe intrusion. (author)

  11. Head-on Quenching of a Non-premixed Flame by an Inert Wall

    NASA Astrophysics Data System (ADS)

    Bharadwaj, Nidheesh

    2005-11-01

    The quenching characteristics of a nonpremixed flame interacting with a wall have been studied via DNS. The vortex ring is generated by a brief discharge of cold methane fuel into hot air. The ignition of the vortex ring is controlled by adjusting the air temperature. The methane combustion has been modeled using detailed kinetic model GRI3.0. The flame is propelled in the axial direction by the ring induced velocity, and interacts head on with a chemically inert isothermal wall. Two wall conditions are examined, one with and one without a thermal boundary layer. The strength of the flame prior to its interaction with the wall is controlled by varying the distance of the wall from the inlet boundary. The effect of the wall on the heat release rate and the structure of the flame is studied. As the flame approaches the wall the magnitudes of vortex ring induced strain rates acting on the flame increase and the maximum wall heat flux occurs on the centerline. It is found that the increase in the strain rates affects the flame power significantly if there is no thermal boundary layer at the wall. Nondimensional wall heat flux, Peclet number, flame structure and near wall reaction mechanisms have been investigated for front flame quenching. For runs with thermal boundary layer, heat released from HO2 reactions is found to be the major contributor to heat flux at the wall.

  12. Evolution equation for the flame surface density in turbulent premixed combustion

    SciTech Connect

    Trouve, A.; Poinsot, T.

    1994-11-01

    An exact evolution equation for the flame surface density, the Sigma-equation, describes the basic physical mechanisms like production by hydrodynamic straining and destruction by propagation effects. Here, direct numerical simulation (DNS) is used to estimate the different terms appearing in the Sigma-equation. The simulations are performed for various mixture Lewis number to modify the strength and nature of the flame-flow coupling. The source and sink terms for the flame surface density are resolved spatially across the turbulent flame brush using the DNS-based analysis. Direct comparisons with flamelet models are also performed. Some areas where the model needs improvement are identified.

  13. The Soret Effect in Naturally Propagating, Premixed, Lean, Hydrogen-Air Flames

    SciTech Connect

    Grcar, Joseph F; Grcar, Joseph F.; Bell, John B.; Day, Marcus S.

    2008-06-30

    Comparatively little attention has been given to multicomponent diffusion effects in lean hydrogen-air flames, in spite of the importance of these flames in safety and their potential importance to future energy technologies. Prior direct numerical simulations either have considered only the mixture-averaged transport model, or have been limited to stabilized flames that do not exhibit the thermo-diffusive instability. The so-called full, multicomponent transport model with cross-diffusion is found to predict hotter, significantly faster flames with much faster extinction and division of cellular structures.

  14. Effects of combined dimension reduction and tabulation on the simulations of a turbulent premixed flame using a large-eddy simulation/probability density function method

    NASA Astrophysics Data System (ADS)

    Kim, Jeonglae; Pope, Stephen B.

    2014-05-01

    A turbulent lean-premixed propane-air flame stabilised by a triangular cylinder as a flame-holder is simulated to assess the accuracy and computational efficiency of combined dimension reduction and tabulation of chemistry. The computational condition matches the Volvo rig experiments. For the reactive simulation, the Lagrangian Large-Eddy Simulation/Probability Density Function (LES/PDF) formulation is used. A novel two-way coupling approach between LES and PDF is applied to obtain resolved density to reduce its statistical fluctuations. Composition mixing is evaluated by the modified Interaction-by-Exchange with the Mean (IEM) model. A baseline case uses In Situ Adaptive Tabulation (ISAT) to calculate chemical reactions efficiently. Its results demonstrate good agreement with the experimental measurements in turbulence statistics, temperature, and minor species mass fractions. For dimension reduction, 11 and 16 represented species are chosen and a variant of Rate Controlled Constrained Equilibrium (RCCE) is applied in conjunction with ISAT to each case. All the quantities in the comparison are indistinguishable from the baseline results using ISAT only. The combined use of RCCE/ISAT reduces the computational time for chemical reaction by more than 50%. However, for the current turbulent premixed flame, chemical reaction takes only a minor portion of the overall computational cost, in contrast to non-premixed flame simulations using LES/PDF, presumably due to the restricted manifold of purely premixed flame in the composition space. Instead, composition mixing is the major contributor to cost reduction since the mean-drift term, which is computationally expensive, is computed for the reduced representation. Overall, a reduction of more than 15% in the computational cost is obtained.

  15. Simultaneous particle image velocimetry and chemiluminescence visualization of millisecond-pulsed current-voltage-induced perturbations of a premixed propane/air flame

    NASA Astrophysics Data System (ADS)

    Schmidt, Jacob; Kostka, Stanislav; Lynch, Amy; Ganguly, Biswa

    2011-09-01

    The effects of millisecond-wide, pulsed current-voltage-induced behavior in premixed laminar flames have been investigated through the simultaneous collection of particle image velocimetry (PIV) and chemiluminescence data with particular attention paid to the onset mechanisms. Disturbances caused by applied voltages of 2 kV over a 30-mm gap to a downward propagating, atmospheric pressure, premixed propane/air flame with a flow speed near 2 m/s and an equivalence ratio of 1.06 are investigated. The combined PIV and chemiluminescence-based experimental data show the observed disturbance originates only in or near the cathode fall region very close to the burner base. The data also suggest that the coupling mechanism responsible for the flame disturbance behavior is fluidic in nature, developing from the radial positive chemi-ion distribution and an ion-drift current-induced net body force that acts along the annular space discharge distribution in the reaction zone in or near the cathode fall. This net body force causes a reduction in flow speed above these near cathodic regions causing the base of the flame to laterally spread. Also, this effect seems to produce a velocity gradient leading to the transition of a laminar flame to turbulent combustion for higher applied current-voltage conditions as shown in previous work (Marcum and Ganguly in Combust Flame 143:27-36, 2005; Schmidt and Ganguly in 48th AIAA aerospace sciences meeting. Orlando, 2010).

  16. effect of hydrogen addition and burner diameter on the stability and structure of lean, premixed flames

    NASA Astrophysics Data System (ADS)

    Kaufman, Kelsey Leigh

    Low swirl burners (LSBs) have gained popularity in heating and gas power generation industries, in part due to their proven capacity for reducing the production of NOx, which in addition to reacting to form smog and acid rain, plays a central role in the formation of the tropospheric ozone layer. With lean operating conditions, LSBs are susceptible to combustion instability, which can result in flame extinction or equipment failure. Extensive work has been performed to understand the nature of LSB combustion, but scaling trends between laboratory- and industrial-sized burners have not been established. Using hydrogen addition as the primary method of flame stabilization, the current work presents results for a 2.54 cm LSB to investigate potential effects of burner outlet diameter on the nature of flame stability, with focus on flashback and lean blowout conditions. In the lean regime, the onset of instability and flame extinction have been shown to occur at similar equivalence ratios for both the 2.54 cm and a 3.81 cm LSB and depend on the resolution of equivalence ratios incremented. Investigations into flame structures are also performed. Discussion begins with a derivation for properties in a multicomponent gas mixture used to determine the Reynolds number (Re) to develop a condition for turbulent intensity similarity in differently-sized LSBs. Based on this requirement, operating conditions are chosen such that the global Reynolds number for the 2.54 cm LSB is within 2% of the Re for the 3.81 cm burner. With similarity obtained, flame structure investigations focus on flame front curvature and flame surface density (FSD). As flame structure results of the current 2.54 cm LSB work are compared to results for the 3.81 cm LSB, no apparent relationship is shown to exist between burner diameter and the distribution of flame surface density. However, burner diameter is shown to have a definite effect on the flame front curvature. In corresponding flow conditions, a

  17. Structure of turbulent non-premixed flames modeled with two-step chemistry

    NASA Technical Reports Server (NTRS)

    Chen, J. H.; Mahalingam, S.; Puri, I. K.; Vervisch, L.

    1992-01-01

    Direct numerical simulations of turbulent diffusion flames modeled with finite-rate, two-step chemistry, A + B yields I, A + I yields P, were carried out. A detailed analysis of the turbulent flame structure reveals the complex nature of the penetration of various reactive species across two reaction zones in mixture fraction space. Due to this two zone structure, these flames were found to be robust, resisting extinction over the parameter ranges investigated. As in single-step computations, mixture fraction dissipation rate and the mixture fraction were found to be statistically correlated. Simulations involving unequal molecular diffusivities suggest that the small scale mixing process and, hence, the turbulent flame structure is sensitive to the Schmidt number.

  18. Premixed hydrogen-oxygen flames. Part II: Quasi-isobaric ignition near the flammability limits

    SciTech Connect

    He, Longting; Clavin, P. Univ. d'Aix-Marseille )

    1993-06-01

    A numerical study of one-dimensional and time-dependent problems in quasi-isobaric combustion of H2-02 mixtures is carried out with a complex chemical network and detailed molecular transport mechanisms. A first numerical result shows that a diffusive-thermal instability corresponding to a Hopf bifurcation appears in the propagation of planar flames in the neighborhood of the H2-rich flammability limit. The corresponding critical mole fraction of H2 is 0.947 at ordinary conditions with a flame velocity of about 45 cm/s, compared with 0.96 for the flammability limit. The quasi-isobaric ignition by a hot pocket of combustion products is also investigated numerically. The critical size of the hot pockets is determined as a function of the equivalence ratio. It is found that when the H2-rich flammability limit is approached, the critical radius becomes much larger than the flame thickness and moreover, it diverges before reaching the planar flammability limit, at a critical H2 mole fraction about 0.945 at ordinary conditions (compared with 0.96). Thus, planar flames cannot be ignited in this way in the range of H2 mole fractions between 0.945 and 0.96 where the burning velocity varies from about 50 cm/s to few millimeters per second. Near the H2 lean flammability limit the situation is quite different. The critical size is smaller than the planar flame thickness, and spherical flames with a very small initial radius may grow in lean mixtures even beyond the flammability limit of planar flames. These phenomena are explained by an elementary analytical study of a minimal model coupling preferential diffusion mechanisms with the kinetic effects controlling the planar flammability limits.

  19. Flame holding tolerant fuel and air premixer for a gas turbine combustor

    DOEpatents

    York, William David; Johnson, Thomas Edward; Ziminsky, Willy Steve

    2012-11-20

    A fuel nozzle with active cooling is provided. It includes an outer peripheral wall, a nozzle center body concentrically disposed within the outer wall in a fuel and air pre-mixture. The fuel and air pre-mixture includes an air inlet, a fuel inlet and a premixing passage defined between the outer wall in the center body. A gas fuel flow passage is provided. A first cooling passage is included within the center body in a second cooling passage is defined between the center body and the outer wall.

  20. Route to chaos for combustion instability in ducted laminar premixed flames

    NASA Astrophysics Data System (ADS)

    Kabiraj, Lipika; Saurabh, Aditya; Wahi, Pankaj; Sujith, R. I.

    2012-06-01

    Complex thermoacoustic oscillations are observed experimentally in a simple laboratory combustor that burns lean premixed fuel-air mixture, as a result of nonlinear interaction between the acoustic field and the combustion processes. The application of nonlinear time series analysis, particularly techniques based on phase space reconstruction from acquired pressure data, reveals rich dynamical behavior and the existence of several complex states. A route to chaos for thermoacoustic instability is established experimentally for the first time. We show that, as the location of the heat source is gradually varied, self-excited periodic thermoacoustic oscillations undergo transition to chaos via the Ruelle-Takens scenario.

  1. The Effect of Gravity on Premixed Flame Propagation and Extinction in a Vertical Standard Flammability Tube

    NASA Technical Reports Server (NTRS)

    Strehlow, Roger A.; Noe, Kurt A.; Wherley, Brian L.

    1988-01-01

    The effect of gravity on the upward and downward flame propagation in lean methane/air and lean propane/air mixtures was studied using plexiglass flammability tubes with ignition at the open-end gravity levels which ranged from microgravity (0 + or - 0.1 g) to 1.77 g. The lean limits were found to be about 5.25, 5.25, and 5.85 percent methane in air; and about 2.15, 2.06, and 2.20 percent propane in air for 1 g upward propagation, 0 g, and 1 g downward propagation, respectively. The propane/air flames observed were stable, irrespective of the g level. On the other hand, lean methane/air flames were found to be sporadically unstable for upward propagation at g levels less than 0.5 g, and for donward propagation at g = 1.0. The extinction process observed was the same for both systems studied: at g = 0, the flame extinguished from the edge toward the center, while at g of 1 and above, the flame extinguished from the center toward the edge.

  2. Premixed flame response to pressure fluctuations using an implicit solver with detailed chemistry

    NASA Astrophysics Data System (ADS)

    Malik, Nadeem

    2015-11-01

    A major challenge in combustion research is the coupling of the compressible flow field to the detailed thermochemistry. Recent advances in numerical solvers has met this challenge within an implicit numerical framework, retaining the full stiffness of the realistic comprehensive chemistry and multicomponent transport properties in the system. Here, the solver TARDIS (Transient Advection Reaction Diffusion Implicit Simulations) is demonstrated, first, by investigating the laminar flame speed in stoichiometric H2/air and CH4/air flames as a function of the flame curvature and found to follow non-linear regimes, contrary to previous thinking. Second, planar and curved laminar flames are subjected to pressure and equivalence ratio oscillations and found to respond through a spectrum of time and length scales. TARDIS has the potential to elucidate fundamental aspects of flame structure and thermochemistry, and could be the basis for a new generation of implicit DNS solvers. The author acknowledge financial support from SABIC, #SB101018, through the Dean of Scientific Research at KFUPM.

  3. Experimental study of Markstein number effects on laminar flamelet velocity in turbulent premixed flames

    SciTech Connect

    Weiss, M.; Zarzalis, N.; Suntz, R.

    2008-09-15

    Effects of turbulent flame stretch on mean local laminar burning velocity of flamelets, u{sub n}, were investigated experimentally in an explosion vessel at normal temperature and pressure. In this context, the wrinkling, A{sub t}/A{sub l}, and the burning velocity, u{sub t}, of turbulent flames were measured simultaneously. With the flamelet assumption the mean local laminar burning velocity of flamelets, u{sub n}=u{sub t} x (A{sub t}/A{sub l}){sup -1}, was calculated for different turbulence intensities. The results were compared to the influence of stretch on spherically expanding laminar flames. For spherically expanding laminar flames the stretched laminar burning velocity, u{sub n}, varied linearly with the Karlovitz stretch factor, yielding Markstein numbers that depend on the mixture composition. Six different mixtures with positive and negative Markstein numbers were investigated. The measurements of the mean local laminar burning velocity of turbulent flamelets were used to derive an efficiency parameter, I, which reflects the impact of the Markstein number and turbulent flame stretch - expressed by the turbulent Karlovitz stretch factor - on the local laminar burning velocity of flamelets. The results showed that the efficiency is reduced with increasing turbulence intensity and the reduction can be correlated to unsteady effects. (author)

  4. Large eddy simulations of partially premixed ethanol dilute spray flames using the flamelet generated manifold model

    NASA Astrophysics Data System (ADS)

    El-Asrag, Hossam A.; Braun, Markus; Masri, Assaad R.

    2016-07-01

    The paper presents Large Eddy Simulations (LESs) for the Sydney ethanol piloted turbulent dilute spray flames ETF2, ETF6, and ETF7. The Flamelet Generated Manifold (FGM) approach is employed to predict mixing and burning of the evaporating fuel droplets. A methodology to match the experimental inflow spray profiles is presented. The spray statistical time-averaged results show reasonable agreement with mean and RMS data. The Particle Size Distribution (PSD) shows a good match downstream of the nozzle exit and up to x/D = 10. At x/D = 20 and 30 the PSD is under-predicted for droplets with mean diameter D10 > 20μm and over-predicted for the smaller size droplets. The simulations reasonably predict the reported mean flame structure and length. The effect of increasing the carrier velocity (ETF2-ETF7) or decreasing the liquid fuel injection mass flow rate (ETF2-ETF6) is found to result in a leaner, shorter flame and stronger spray-flow interactions. Higher tendency to local extinction is observed for ETF7 which is closer to blow-off compared to ETF2 and has higher scalar dissipation rates, higher range of Stokes number, and faster droplet response. The possible sources of LES-FGM deviations from the measurements are discussed and highlighted. In particular, the spray time-averaged statistical error contribution is quantified and the impact of the inflow uncertainty is studied. Sensitivity analysis to the pre-vaporized nozzle fuel mass fraction show that such small inflow perturbations (by ± 2% for the ETF2 flame) have a strong impact on the flame structure, and the droplets' dynamics. Conditional scatter plots show that the flame exhibits wide range of mixing conditions and bimodal mixing lines particularly at upstream locations (x/D < 20), where the injected droplets are still penetrating the centerline. This is relaxed further downstream as droplets gradually evaporate and burn in a diffusion like mode.

  5. Diffusive-thermal oscillations of rich premixed hydrogen-air flames in a microflow reactor

    NASA Astrophysics Data System (ADS)

    Miroshnichenko, Taisia; Gubernov, Vladimir; Maruta, Kaoru; Minaev, Sergei

    2016-03-01

    In this paper the dynamics of rich hydrogen-air flames in a microflow reactor with controlled temperature of the walls is investigated numerically using the thermal-diffusion model with two-step kinetics in one spatial dimension. It is found that as the parameters of the system are varied the sequence of bifurcation occurs leading to the formation of complex spatio-temporal patterns. These include pulsating, chaotic, mixed-mode and FREI (Flames with Repetitive Extinction and Ignition) oscillations. The critical parameter values for the existence of different dynamical regimes are found in terms of equivalence ratio and flow velocity.

  6. Mixing and stabilization study of a partially premixed swirling flame using laser induced fluorescence

    SciTech Connect

    Galley, D.; Ducruix, S.; Lacas, F.; Veynante, D.

    2011-01-15

    A laboratory-scale swirling burner, presenting many similarities with gas turbines combustors, has been studied experimentally using planar laser induced fluorescence (PLIF) on OH radical and acetone vapor in order to characterize the flame stabilization process. These diagnostics show that the stabilization point rotates in the combustion chamber and that air and fuel mixing is not complete at the end of the mixing tube. Fuel mass fraction decays exponentially along the mixing tube axis and transverse profiles show a gaussian shape. However, radial pressure gradients tend to trap the fuel in the core of the vortex that propagates axially in the mixing tube. As the mixing tube vortex enters the combustion chamber, vortex breakdown occurs through a precessing vortex core (PVC). The axially propagating vortex shows a helicoidal trajectory in the combustion chamber which trace is observed with transverse acetone PLIF. As a consequence, the stabilizing point of the flame in the combustion chamber rotates with the PVC structure. This phenomenon has been observed in the present study with a high speed camera recording spontaneous emission of the flame. The stabilization point rotation frequency tends to increase with mass flow rates. It was also shown that the coupling between the PVC and the flame stabilization occurs via mixing, explaining one possible coupling mechanism between acoustic waves in the flow and the reaction rate. This path may also be envisaged for flashback, an issue that will be more completely treated in a near future. (author)

  7. An experimental study of the velocity-forced flame response of a lean-premixed multi-nozzle can combustor for gas turbines

    NASA Astrophysics Data System (ADS)

    Szedlmayer, Michael Thomas

    The velocity forced flame response of a multi-nozzle, lean-premixed, swirl-stabilized, turbulent combustor was investigated at atmospheric pressure. The purpose of this study was to analyze the mechanisms that allowed velocity fluctuations to cause fluctuations in the rate of heat release in a gas turbine combustor experiencing combustion instability. Controlled velocity fluctuations were introduced to the combustor by a rotating siren device which periodically allowed the air-natural gas mixture to flow. The velocity fluctuation entering the combustor was measured using the two-microphone method. The resulting heat release rate fluctuation was measured using CH* chemiluminescence. The global response of the flame was quantified using the flame transfer function with the velocity fluctuation as the input and the heat release rate fluctuation as the output. Velocity fluctuation amplitude was initially maintained at 5% of the inlet velocity in order to remain in the linear response regime. Flame transfer function measurements were acquired at a wide range of operating conditions and forcing frequencies. The selected range corresponds to the conditions and instability frequencies typical of real gas turbine combustors. Multi-nozzle flame transfer functions were found to bear a qualitative similarity to the single-nozzle flame transfer functions in the literature. The flame transfer function gain exhibited alternating minima and maxima while the phase decreased linearly with increasing forcing frequency. Several normalization techniques were applied to all flame transfer function data in an attempt to collapse the data into a single curve. The best collapse was found to occur using a Strouhal number which was the ratio of the characteristic flame length to the wavelength of the forced disturbance. Critical values of Strouhal number are used to predict the shedding of vortical structures in shear layers. Because of the collapse observed when the flame transfer functions

  8. Extinction of premixed flames of practical liquid fuels: Experiments and simulations

    SciTech Connect

    Holley, A.T.; Dong, Y.; Andac, M.G.; Egolfopoulos, F.N.

    2006-02-01

    Compared to those for gaseous fuels, fundamental flame studies for liquid fuels are less extensive. The reasons are the experimental difficulty in handling the liquid phase and the complexity of kinetics stemming from the structure of liquid fuel molecules. However, such fuels are important in power generation, transportation, and propulsion. In this investigation, a systematic study has been conducted on the extinction of mixtures of methanol, ethanol, n-heptane, and iso-octane with air. The experiments were performed in the counterflow configuration and the extinction strain rates were determined through the use of digital particle image velocimetry. The introduction of the liquid fuel into the air was achieved through a liquid fuel feeder. The liquid flow rates were determined through the use of a high-precision pump. The experiments were conducted at ambient pressure and temperature and the maximum achievable equivalence ratios were limited by the attendant vapor pressure of each liquid fuel. The experiments were numerically simulated using detailed descriptions of chemical kinetic and molecular transport. A number of kinetic mechanisms were tested against the experimentally determined extinction strain rates. The mechanisms were also tested against literature data of laminar flame speeds. It was found that while most mechanisms satisfactorily predict laminar flame speeds, the experimental and predicted extinction strain rates can differ by factors of as much as 2 to 3. Under certain conditions, distinct differences were identified in the kinetic pathways that control the phenomena of propagation and extinction. Additionally, it was found that the sensitivity of laminar flame speeds and extinction strain rates to diffusion could be of the same order as that to kinetics. (author)

  9. Gaseous Non-Premixed Flame Research Planned for the International Space Station

    NASA Technical Reports Server (NTRS)

    Stocker, Dennis P.; Takahashi, Fumiaki; Hickman, J. Mark; Suttles, Andrew C.

    2014-01-01

    Thus far, studies of gaseous diffusion flames on the International Space Station (ISS) have been limited to research conducted in the Microgravity Science Glovebox (MSG) in mid-2009 and early 2012. The research was performed with limited instrumentation, but novel techniques allowed for the determination of the soot temperature and volume fraction. Development is now underway for the next experiments of this type. The Advanced Combustion via Microgravity Experiments (ACME) project consists of five independent experiments that will be conducted with expanded instrumentation within the stations Combustion Integrated Rack (CIR). ACMEs goals are to improve our understanding of flame stability and extinction limits, soot control and reduction, oxygen-enriched combustion which could enable practical carbon sequestration, combustion at fuel lean conditions where both optimum performance and low emissions can be achieved, the use of electric fields for combustion control, and materials flammability. The microgravity environment provides longer residence times and larger length scales, yielding a broad range of flame conditions which are beneficial for simplified analysis, e.g., of limit behaviour where chemical kinetics are important. The detailed design of the modular ACME hardware, e.g., with exchangeable burners, is nearing completion, and it is expected that on-orbit testing will begin in 2016.

  10. Apparatus for studying premixed laminar flames using mass spectrometry and fiber-optic spectrometry

    NASA Astrophysics Data System (ADS)

    Olsson, Jim O.; Andersson, Lars L.; Lenner, Magnus; Simonson, Margaret

    1990-03-01

    An integrated flat-flame/ microprobe sampling quadrupole mass spectrometer system, complemented by optical spectrometry based on optical fibers, is presented. The short microprobe sampling line (total 25 cm) is directly connected to an open ion source closely flanked by two nude cryopumps (900 l/s) yielding a background pressure of 10-9 Torr and a sampling pressure of about 10-5 Torr. Due to this improved microprobe system, mass spectrometry can be used for analysis of stable species (including fuel, O2, H2O, CO2, CO, and Ar) with less disturbance of the sample than with a conventional microprobe with a back pressure of about 1 Torr. Optical spectrometry is used for the study of emission from important radical species (such as C2, CH, and OH). The system is proposed as a complement to more conventional flat-flame/MBMS systems in which the sampling cone can effect the experimental system. Details are provided concerning the configuration of the whole system ranging from gas delivery to data evaluation. Test data are presented for a 16% methanol/68% oxygen/16% argon flame studied at a pressure of 40 Torr, to elucidate the special features of this system.

  11. Simultaneous one-dimensional fluorescence lifetime measurements of OH and CO in premixed flames

    NASA Astrophysics Data System (ADS)

    Jonsson, Malin; Ehn, Andreas; Christensen, Moah; Aldén, Marcus; Bood, Joakim

    2014-04-01

    A method for simultaneous measurements of fluorescence lifetimes of two species along a line is described. The experimental setup is based on picosecond laser pulses from two tunable optical parametric generator/optical parametric amplifier systems together with a streak camera. With an appropriate optical time delay between the two laser pulses, whose wavelengths are tuned to excite two different species, laser-induced fluorescence can be both detected temporally and spatially resolved by the streak camera. Hence, our method enables one-dimensional imaging of fluorescence lifetimes of two species in the same streak camera recording. The concept is demonstrated for fluorescence lifetime measurements of CO and OH in a laminar methane/air flame on a Bunsen-type burner. Measurements were taken in flames with four different equivalence ratios, namely ϕ = 0.9, 1.0, 1.15, and 1.25. The measured one-dimensional lifetime profiles generally agree well with lifetimes calculated from quenching cross sections found in the literature and quencher concentrations predicted by the GRI 3.0 mechanism. For OH, there is a systematic deviation of approximately 30 % between calculated and measured lifetimes. It is found that this is mainly due to the adiabatic assumption regarding the flame and uncertainty in H2O quenching cross section. This emphasizes the strength of measuring the quenching rates rather than relying on models. The measurement concept might be useful for single-shot measurements of fluorescence lifetimes of several species pairs of vital importance in combustion processes, hence allowing fluorescence signals to be corrected for quenching and ultimately yield quantitative concentration profiles.

  12. Numerical simulation and sensitivity analysis of detailed soot particle size distribution in laminar premixed ethylene flames

    SciTech Connect

    Singh, Jasdeep; Patterson, Robert I.A.; Kraft, Markus; Wang, Hai

    2006-04-15

    In this paper, the prediction of a soot model [J. Appel, H. Bockhorn, M. Frenklach, Combust. Flame 121 (2000) 122-136] is compared to a recently published set of highly detailed soot particle size distributions [B. Zhao, Z. Yang, Z. Li, M.V. Johnston, H. Wang, Proc. Combust. Inst. 30 (2005)]. A stochastic approach is used to obtain soot particle size distributions (PSDs). The key features of the measured and simulated particle size distributions are identified and used as a simple way of comparing PSDs. The sensitivity of the soot PSDs to the parameters defining parts of the soot model, such as soot inception, particle and PAH collision efficiency and enhancement, and surface activity is investigated. Incepting soot particle size is found to have a very significant effect on the small-size end of the PSDs, especially the position of the trough for a bimodal soot PSDs. A new model for the decay in the surface activity is proposed in which the activity of the soot particle depends only on the history of that particle and the local temperature in the flame. This is a first attempt to use local flame variables to define the surface aging which has major impact on the prediction of the large-size end of the PSDs. Using these modifications to the soot model it is possible to improve the agreement between some of the points of interest in the simulated and measured PSDs. The paper achieves the task to help advance the soot models to predict soot PSD in addition to soot volume fraction and number density, which has been the focus of the literature. (author)

  13. Verification and Improvement of Flamelet Approach for Non-Premixed Flames

    NASA Technical Reports Server (NTRS)

    Zaitsev, S.; Buriko, Yu.; Guskov, O.; Kopchenov, V.; Lubimov, D.; Tshepin, S.; Volkov, D.

    1997-01-01

    Studies in the mathematical modeling of the high-speed turbulent combustion has received renewal attention in the recent years. The review of fundamentals, approaches and extensive bibliography was presented by Bray, Libbi and Williams. In order to obtain accurate predictions for turbulent combustible flows, the effects of turbulent fluctuations on the chemical source terms should be taken into account. The averaging of chemical source terms requires to utilize probability density function (PDF) model. There are two main approaches which are dominant in high-speed combustion modeling now. In the first approach, PDF form is assumed based on intuitia of modelliers (see, for example, Spiegler et.al.; Girimaji; Baurle et.al.). The second way is much more elaborate and it is based on the solution of evolution equation for PDF. This approach was proposed by S.Pope for incompressible flames. Recently, it was modified for modeling of compressible flames in studies of Farschi; Hsu; Hsu, Raji, Norris; Eifer, Kollman. But its realization in CFD is extremely expensive in computations due to large multidimensionality of PDF evolution equation (Baurle, Hsu, Hassan).

  14. Visualization and Analysis of a Hydrocarbon Premixed Flame a in Small Scale Scramjet Combustor

    NASA Astrophysics Data System (ADS)

    Cantu, Luca Maria Luigi

    Nitric oxide (NO) planar induced laser fluorescence (PLIF) measurements have been performed in a small scale scramjet combustor at the University of Virginia Aerospace Research Laboratory at nominal simulated Mach 5 flight enthalpy. A mixture of NO and N2 was injected at the upstream end of the inlet isolator as a surrogate for ethylene fuel, and the mixing of this fuel simulant was studied with and without a shock train. The shock train was produced by an air throttle, which simulated the blockage effects of combustion downstream of the cavity flame holder. NO PLIF signal was imaged in a plane orthogonal to the freestream at the leading edge of the cavity. Instantaneous planar images were recorded and analyzed to identify the most uniform cases, which were achieved by varying the location of the fuel injection and shock train. This method was used to screen different possible fueling configurations to provide optimized test conditions for follow-on combustion measurements using ethylene fuel. A theoretical study of the selected NO rotational transitions was performed to obtain a LIF signal that is linear with NO mole fraction and approximately independent of pressure and temperature. In the same facility, OH PLIF measurements were also performed; OH lines were carefully chosen to have fluorescent signal that is independent of pressure and temperature but linear with mole fraction. The OH PLIF signal was imaged in planes orthogonal to and parallel to the freestream flow at different equivalence ratios. Flameout limits were tested and identified. Instantaneous planar images were recorded and analyzed to compare the results with width increased dual-pump enhanced coherent anti-Stokes Raman spectroscopy (WIDECARS) measurements in the same facility and large eddy simulation/Reynolds average Navier-Stokes (LES/RANS) numerical simulations. The flame angle was found to be approximately 10 degrees for several different conditions, which is in agreement with numerical

  15. Premixed Atmosphere and Convection Influences on Flame Inhibition and Combustion (PACIFIC)

    NASA Technical Reports Server (NTRS)

    Ronney, Paul D.

    1995-01-01

    Under NASA-Lewis Grant NAG3-1611, starting date 6/1/94, a three-year experimental and theoretical study of the effects of ambient atmosphere on the properties of flame spread over thin and thick solid fuel beds has been initiated. In particular the effect of the type of inert gas, which affects the Lewis numbers of fuel and oxidant, and the effect of the addition of sub-flammability-limit concentrations of gaseous fuels to the oxidizing atmosphere will be studied. The effect of convection will be studied through one-g and mu g experiments with and without a forced flow. Moreover, the influence of thermal radiation, whose effect is known to be markedly different depending on the convection level, will be addressed.

  16. Extinction measurements for optical band gap determination of soot in a series of nitrogen-diluted ethylene/air non-premixed flames.

    PubMed

    Adkins, Erin M; Miller, J Houston

    2015-01-28

    Visible light extinction was measured in a series of nitrogen-diluted, ethylene/air, non-premixed flames and this data was used to determine the optical band gap, OBG, as a function of flame position. Collimated light from a supercontinuum source is telescopically expanded and refocused to match the f- number of a dispersing monochromator. The dispersed light is split into a power metering channel and a channel that is periscoped and focused into the flame. The transmitted light is then recollimated and focussed onto a silicon photodiode detector. After tomographic reconstruction of the radial extinction field, the OBG was derived from the near-edge absorption feature using Tauc/Davis-Mott analysis. A slight evolution in OBG was observed throughout all flame systems with a consistent range of OBG observed between approximately 1.85 eV and 2.35 eV. Averaging over all positions the mean OBG was approximately 2.09 eV for all flame systems. Comparing these results to previously published computational results relating calculated HOMO-LUMO gaps for a variety of D2h PAH molecules to the number of aromatic rings in the structure, showed that the observed optical band gap is consistent with a PAH of about 14 rings or a conjugation length of 0.97 nm. This work provides experimental support to the model of soot formation where the transition from chemical to physical growth starts at a modest molecular size; about the size of circumpyrene.

  17. Semi-analytical emission model for diffusion flame, rich/lean and premixed lean combustors

    NASA Astrophysics Data System (ADS)

    Rizk, N. K.; Mongia, H. C.

    1995-04-01

    To enhance gas turbine combustor performance and emissions characteristics, better design methods need to be developed. In the present investigation, an emission model that simulates a detailed chemical kinetic scheme has been developed to provide the rate of reactions of the parent fuel, an intermediate hydrocarbon compound, CO, and H2. The intermediate fuel has variable carbon and hydrogen contents depending on operating conditions, that were selected in the development effort to simulate actual operation of rich/lean, diffusion flame, and lean combustor concepts. The developed reaction rate expressions address also the limited reaction rates that may occur in the near-wall regions of the combustor due to the admittance of radial air jets and cooling air in these regions. The validation effort included the application of the developed model to a combustor simulated by a multiple-reactor arrangement. The results indicate the accurate duplication of the calculations obtained from the detailed kinetic scheme using the developed model. This illustrates the great potential of using such a unified approach to guide the design of various types of combustor to meet the more stringent emissions and performance requirements of next-generation gas turbine engines.

  18. A lean methane premixed laminar flame doped with components of diesel fuel part III: Indane and comparison between n-butylbenzene, n-propylcyclohexane and indane

    SciTech Connect

    Pousse, E.; Tian, Z.Y.; Glaude, P.A.; Fournet, R.; Battin-Leclerc, F.

    2010-07-15

    To better understand the chemistry of the combustion of components of diesel fuel, the structure of a laminar lean premixed methane flame doped with indane has been investigated. The inlet gases contained 7.1% (molar) of methane, 36.8% of oxygen and 0.9% of indane corresponding to an equivalence ratio of 0.67 and a ratio C{sub 10}H{sub 14}/CH{sub 4} of 12.8%. The flame has been stabilized on a burner at a pressure of 6.7 kPa (50 Torr) using argon as diluent, with a gas velocity at the burner of 49.1 cm s{sup -1} at 333 K. Quantified species included the usual methane C{sub 0}-C{sub 2} combustion products, but also 16 C{sub 3}-C{sub 5} non-aromatic hydrocarbons, 6 C{sub 1}-C{sub 3} non-aromatic oxygenated compounds, as well as 22 aromatic products, namely benzene, toluene, xylenes, phenylacetylene, ethylbenzene, styrene, propenylbenzene, allylbenzene, n-propylbenzene, methylstyrenes, ethyltoluenes, trimethylbenzenes, n-butylbenzene, dimethylethylbenzene, indene, methylindenes, methylindane, benzocyclobutene, naphthalene, phenol, benzaldehyde, and benzofuran. A new mechanism for the oxidation of indane was proposed whose predictions were in satisfactory agreement with measured species profiles in both flames and jet-stirred reactor experiments. The main reaction pathways of consumption of indane have been derived from flow rate analyses in the two types of reactors. A comparison of the effect of the addition of three components of diesel fuel, namely indane, n-butylbenzene and n-propylcyclohexane (parts I and II of this series of paper), on the structure of a laminar lean premixed methane flame is also presented. (author)

  19. Electrical Characteristics, Electrode Sheath and Contamination Layer Behavior of a Meso-Scale Premixed Methane-Air Flame Under AC/DC Electric Fields

    NASA Astrophysics Data System (ADS)

    Chen, Qi; Yan, Limin; Zhang, Hao; Li, Guoxiu

    2016-05-01

    Electrical characteristics of a nozzle-attached meso-scale premixed methane-air flame under low-frequency AC (0-4300 V, 0-500 Hz) and DC (0-3300 V) electric fields were studied. I-V curves were measured under different experimental conditions to estimate the magnitude of the total current 100-102 μA, the electron density 1015-1016 m-3 and further the power dissipation ≤ 0.7 W in the reaction zone. At the same time, the meso-scale premixed flame conductivity 10-4-10-3 Ω-1·m-1 as a function of voltage and frequency was experimentally obtained and was believed to represent a useful order-of magnitude estimate. Moreover, the influence of the collision sheath relating to Debye length (31-98 μm) and the contamination layer of an active electrode on measurements was discussed, based on the combination of simulation and theoretical analysis. As a result, the electrode sheath dimension was evaluated to less than 0.5 mm, which indicated a complex effect of the collision sheath on the current measurements. The surface contamination effect of an active electrode was further analyzed using the SEM imaging method, which showed elements immigration during the contamination layer formation process. supported by National Natural Science Foundation of China (No. 51376021), and the Fundamental Research Fund for Major Universities (No. 2013JBM079)

  20. Electrical Characteristics, Electrode Sheath and Contamination Layer Behavior of a Meso-Scale Premixed Methane-Air Flame Under AC/DC Electric Fields

    NASA Astrophysics Data System (ADS)

    Chen, Qi; Yan, Limin; Zhang, Hao; Li, Guoxiu

    2016-05-01

    Electrical characteristics of a nozzle-attached meso-scale premixed methane-air flame under low-frequency AC (0-4300 V, 0-500 Hz) and DC (0-3300 V) electric fields were studied. I-V curves were measured under different experimental conditions to estimate the magnitude of the total current 100-102 μA, the electron density 1015-1016 m‑3 and further the power dissipation ≤ 0.7 W in the reaction zone. At the same time, the meso-scale premixed flame conductivity 10‑4-10‑3 Ω‑1·m‑1 as a function of voltage and frequency was experimentally obtained and was believed to represent a useful order-of magnitude estimate. Moreover, the influence of the collision sheath relating to Debye length (31–98 μm) and the contamination layer of an active electrode on measurements was discussed, based on the combination of simulation and theoretical analysis. As a result, the electrode sheath dimension was evaluated to less than 0.5 mm, which indicated a complex effect of the collision sheath on the current measurements. The surface contamination effect of an active electrode was further analyzed using the SEM imaging method, which showed elements immigration during the contamination layer formation process. supported by National Natural Science Foundation of China (No. 51376021), and the Fundamental Research Fund for Major Universities (No. 2013JBM079)

  1. Turbulence and combustion interaction: High resolution local flame front structure visualization using simultaneous single-shot PLIF imaging of CH, OH, and CH{sub 2}O in a piloted premixed jet flame

    SciTech Connect

    Li, Z.S.; Li, B.; Sun, Z.W.; Alden, M.; Bai, X.S.

    2010-06-15

    High resolution planar laser-induced fluorescence (PLIF) was applied to investigate the local flame front structures of turbulent premixed methane/air jet flames in order to reveal details about turbulence and flame interaction. The targeted turbulent flames were generated on a specially designed coaxial jet burner, in which low speed stoichiometric gas mixture was fed through the outer large tube to provide a laminar pilot flame for stabilization of the high speed jet flame issued through the small inner tube. By varying the inner tube flow speed and keeping the mixture composition as that of the outer tube, different flames were obtained covering both the laminar and turbulent flame regimes with different turbulent intensities. Simultaneous CH/CH{sub 2}O, and also OH PLIF images were recorded to characterize the influence of turbulence eddies on the reaction zone structure, with a spatial resolution of about 40 {mu}m and temporal resolution of around 10 ns. Under all experimental conditions, the CH radicals were found to exist only in a thin layer; the CH{sub 2}O were found in the inner flame whereas the OH radicals were seen in the outer flame with the thin CH layer separating the OH and CH{sub 2}O layers. The outer OH layer is thick and it corresponds to the oxidation zone and post-flame zone; the CH{sub 2}O layer is thin in laminar flows; it becomes broad at high speed turbulent flow conditions. This phenomenon was analyzed using chemical kinetic calculations and eddy/flame interaction theory. It appears that under high turbulence intensity conditions, the small eddies in the preheat zone can transport species such as CH{sub 2}O from the reaction zones to the preheat zone. The CH{sub 2}O species are not consumed in the preheat zone due to the absence of H, O, and OH radicals by which CH{sub 2}O is to be oxidized. The CH radicals cannot exist in the preheat zone due to the rapid reactions of this species with O{sub 2} and CO{sub 2} in the inner-layer of the

  2. Temporally resolved planar measurements of transient phenomena in a partially pre-mixed swirl flame in a gas turbine model combustor

    SciTech Connect

    Boxx, I.; Stoehr, M.; Meier, W.; Carter, C.

    2010-08-15

    This paper presents observations and analysis of the time-dependent behavior of a 10 kW partially pre-mixed, swirl-stabilized methane-air flame exhibiting self-excited thermo-acoustic oscillations. This analysis is based on a series of measurements wherein particle image velocimetry (PIV) and planar laser-induced fluorescence (PLIF) of the OH radical were performed simultaneously at 5 kHz repetition rate over durations of 0.8 s. Chemiluminescence imaging of the OH{sup *} radical was performed separately, also at 5 kHz over 0.8 s acquisition runs. These measurements were of sufficient sampling frequency and duration to extract usable spatial and temporal frequency information on the medium to large-scale flow-field and heat-release characteristics of the flame. This analysis is used to more fully characterize the interaction between the self-excited thermo-acoustic oscillations and the dominant flow-field structure of this flame, a precessing vortex core (PVC) present in the inner recirculation zone. Interpretation of individual measurement sequences yielded insight into various physical phenomena and the underlying mechanisms driving flame dynamics. It is observed for this flame that location of the reaction zone tracks large-scale fluctuations in axial velocity and also conforms to the passage of large-scale vortical structures through the flow-field. Local extinction of the reaction zone in regions of persistently high principal compressive strain is observed. Such extinctions, however, are seen to be self healing and thus do not induce blowout. Indications of auto-ignition in regions of unburned gas near the exit are also observed. Probable auto-ignition events are frequently observed coincident with the centers of large-scale vortical structures, suggesting the phenomenon is linked to the enhanced mixing and longer residence times associated with fluid at the core of the PVC as it moves through the flame. (author)

  3. Turbulent burning velocities of premixed CH{sub 4}/diluent/air flames in intense isotropic turbulence with consideration of radiation losses

    SciTech Connect

    Shy, S.S.; Yang, S.I.; Lin, W.J.; Su, R.C.

    2005-10-01

    This paper presents turbulent burning velocities, S{sub T}, of several premixed CH{sub 4}/diluent/air flames at the same laminar burning velocity S{sub L}=0.1 m/s for two equivalence ratios f=0.7 and 1.4 near flammability limits with consideration of radiation heat losses from small (N{sub 2} diluted) to large (CO{sub 2} diluted). Experiments are carried out in a cruciform burner, in which the long vertical vessel is used to provide a downward propagating premixed flame and the large horizontal vessel equipped with a pair of counterrotating fans and perforated plates can be used to generate an intense isotropic turbulence in the central region between the two perforated plates. Turbulent flame speeds are measured by four different arrangements of pairs of ion-probe sensors at different positions from the top to the bottom of the central region in the burner. It is found that the effect of gas velocity on S{sub T} measured in the central region can be neglected. Simultaneous measurements using the pressure transducer and ion-probe sensors show that the pressure rise due to turbulent burning has little influence on S{sub T}. These measurements prove the accuracy of the S{sub T} data. At f=0.7, the percentage of [(S{sub T}/S{sub L}){sub CO{sub 2}}-(S{sub T}/S{sub L}){sub N{sub 2}}]/(S{sub T}/S{sub L}){sub N{sub 2}} decreases gradually from -4 to -17% when values of u{sup '}/S{sub L} increase from 4 to 46, while at f=1.4 such decrease is much more abrupt from -19 to -53% when values of u{sup '}/S{sub L} only increase from 4 to 18. The larger the radiation losses, the smaller the values of S{sub T}. This decreasing effect is augmented by increasing u{sup '}/S{sub L} and is particularly pronounced for rich CH{sub 4} flames. When u{sup '}/S{sub L}=18, lean CO{sub 2} and/or N{sub 2}-diluted CH{sub 4} flames have much higher, 3.6 and/or 1.8 times higher, values of S{sub T}/S{sub L} than rich CO{sub 2} and/or N{sub 2}-diluted CH{sub 4} flames, respectively. It is found that

  4. Kinetic parameters, collision rates, energy exchanges and transport coefficients of non-thermal electrons in premixed flames at sub-breakdown electric field strengths

    NASA Astrophysics Data System (ADS)

    Bisetti, Fabrizio; El Morsli, Mbark

    2014-01-01

    The effects of an electric field on the collision rates, energy exchanges and transport properties of electrons in premixed flames are investigated via solutions to the Boltzmann kinetic equation. The case of high electric field strength, which results in high-energy, non-thermal electrons, is analysed in detail at sub-breakdown conditions. The rates of inelastic collisions and the energy exchange between electrons and neutrals in the reaction zone of the flame are characterised quantitatively. The analysis includes attachment, ionisation, impact dissociation, and vibrational and electronic excitation processes. Our results suggest that Townsend breakdown occurs for E/N = 140 Td. Vibrational excitation is the dominant process up to breakdown, despite important rates of electronic excitation of CO, CO2 and N2 as well as impact dissociation of O2 being apparent from 50 Td onwards. Ohmic heating in the reaction zone is found to be negligible (less than 2% of peak heat release rate) up to breakdown field strengths for realistic electron densities equal to 1010 cm-3. The observed trends are largely independent of equivalence ratio. In the non-thermal regime, electron transport coefficients are insensitive to mixture composition and approximately constant across the flame, but are highly dependent on the electric field strength. In the thermal limit, kinetic parameters and transport coefficients vary substantially across the flame due to the spatially inhomogeneous concentration of water vapour. A practical approach for identifying the plasma regime (thermal versus non-thermal) in studies of electric field effects on flames is proposed.

  5. Quantitative Studies on the Propagation and Extinction of Near-Limit Premixed Flames under Normal- and Micro-gravity

    NASA Technical Reports Server (NTRS)

    Egolfopoulos, F. N.; Dong, Y.; Spedding, G.; Cuenot, B.; Poinsot, T.

    2001-01-01

    Strained laminar flames have been systematically studied, as the understanding of their structure and dynamic behavior is of relevance to turbulent combustion.. Most of these studies have been conducted in opposed-jet, stagnation-type flow configurations. Studies at high strain rates are important in quantifying and understanding the response of vigorously burning flames and determine extinction states. Studies of weakly strained flames can be of particular interest for all stoichiometries. For example, the laminar flame speeds, S(sup o)(sub u), can be accurately determined by using the counterflow technique only if measurements are obtained at very low strain rates. Furthermore, near-limit flames are stabilized by weak strain rates. Previous studies have shown that near-limit flames are particularly sensitive to chain mechanisms, thermal radiation, and unsteadiness. The stabilization and study of weakly strained flames is complicated by the presence of buoyancy that can render the flames unstable to the point of extinction. Thus, the use of microgravity (mu-g) becomes essential in order to provide meaningful insight into this important combustion regime. In our past studies the laminar flame speeds and extinction strain rates were directly measured at ultra-low strain rates. The laminar flame speeds were measured by having a positively strained planar flame undergoing a transition to a negatively strained Bunsen flame and by measuring the propagation speed during that transition. The extinction strain rates of near-limit flames were measured in mu-g. Results obtained for CH4/air and C3H8/air mixtures are in agreement with those obtained by Maruta et al.

  6. The behavior of fuel-lean premixed flames in a standard flammability limit tube under controlled gravity conditions

    NASA Technical Reports Server (NTRS)

    Wherley, B. L.; Strehlow, R. A.

    1986-01-01

    Fuel-lean flames in methane-air mixtures from 4.90 to 6.20 volume percent fuel and propane-air mixtures from 1.90 to 3.00 volume percent fuel were studied in the vicinity of the limit for a variety of gravity conditions. The limits were determined and the behavior of the flames studied for one g upward, one g downward, and zero g propagation. Photographic records of all flammability tube firings were obtained. The structure and behavior of these flames were detailed including the variations of the curvature of the flame front, the skirt length, and the occurrence of cellular instabilities with varying gravity conditions. The effect of ignition was also discussed. A survey of flame speeds as a function of mixture strength was made over a range of lean mixture compositions for each of the fuels studied. The results were presented graphically with those obtained by other researchers. The flame speed for constant fractional gravity loadings were plotted as a function of gravity loadings from 0.0 up to 2.0 g's against flame speeds extracted from the transient gravity flame histories for corresponding gravity loadings. The effects of varying gravity conditions on the extinguishment process for upward and downward propagating flames were investigated.

  7. Studies in premixed combustion. Progress report, November 1, 1990--October 31, 1992

    SciTech Connect

    Sivashinsky, G.I.

    1992-08-01

    This report discusses the following topics on premixed combustion: theory of turbulent flame propagation; pattern formation in premixed flames and related problems; and pattern formation in extended systems. (LSP)

  8. Asymptotic expressions for turbulent burning velocity at the leading edge of a premixed flame brush and their validation by published measurement data

    NASA Astrophysics Data System (ADS)

    Lee, Jaeseo; Lee, Gwang G.; Huh, Kang Y.

    2014-12-01

    This paper presents validation of new analytical expressions for the turbulent burning velocity, ST, based on asymptotic behavior at the leading edge (LE) in turbulent premixed combustion. Reaction and density variation are assumed to be negligible at the LE to avoid the cold boundary difficulty in the statistically steady state. Good agreement is shown for the slopes, dST/du', with respect to Lc/δf at low turbulence, with both normalized by those of the reference cases. δf is the inverse of the maximum gradient of reaction progress variable through an unstretched laminar flame, and Lc is the characteristic length scale given as burner diameter or measured integral length scale. Comparison is made for thirty-five datasets involving different fuels, equivalence ratios, H2 fractions in fuel, pressures, and integral length scales from eight references [R. C. Aldredge et al., "Premixed-flame propagation in turbulent Taylor-Couette flow," Combust. Flame 115, 395 (1998); M. Lawes et al., "The turbulent burning velocity of iso-octane/air mixtures," Combust. Flame 159, 1949 (2012); H. Kido et al., "Influence of local flame displacement velocity on turbulent burning velocity," Proc. Combust. Inst. 29, 1855 (2002); J. Wang et al., "Correlation of turbulent burning velocity for syngas/air mixtures at high pressure up to 1.0 MPa," Exp. Therm. Fluid Sci. 50, 90 (2013); H. Kobayashi et al., "Experimental study on general correlation of turbulent burning velocity at high pressure," Proc. Combust. Inst. 27, 941 (1998); C. W. Chiu et al., "High-pressure hydrogen/carbon monoxide syngas turbulent burning velocities measured at constant turbulent Reynolds numbers," Int. J. Hydrogen Energy 37, 10935 (2012); P. Venkateswaran et al., "Pressure and fuel effects on turbulent consumption speeds of H2/CO blends," Proc. Combust. Inst. 34, 1527 (2013); M. Fairweather et al., "Turbulent burning rates of methane and methane-hydrogen mixtures," Combust. Flame 156, 780 (2009)]. The turbulent

  9. Premixed flames in stagnating turbulence. Part VI. Predicting the mean density and the permitted rates of strain for impinging reactant streams

    SciTech Connect

    Bray, Ken; Champion, Michel; Libby, Paul A.

    2009-02-15

    A RANS analysis of a jet of premixed reactants impinging on a wall is presented. Unlike previous related studies by the same authors, in which the mean density distribution through the flame brush is specified from experiment in order to concentrate on the fluid mechanics of the problem, the mean density is computed in the present work. As a consequence, an appropriate description for the mean rate of heat release is required. The presumed PDF model selected for this purpose, with strong support from relevant DNS, is supplemented with a new model for the mean scalar dissipation rate. Illustrative numerical results are presented and it is shown that an approximately sixfold increase in a mean strain rate function is required to displace the flame from a location where flashback to the nozzle is about to occur to a position so close to the wall that extinction is imminent. Comparisons of predicted mean property distributions with published experimental data are found to be satisfactory and to lend support to the proposed model. (author)

  10. Evolution of soot size distribution in premixed ethylene/air and ethylene/benzene/air flames: Experimental and modeling study

    SciTech Connect

    Echavarria, Carlos A.; Sarofim, Adel F.; Lighty, JoAnn S.; D'Anna, Andrea

    2011-01-15

    The effect of benzene concentration in the initial fuel on the evolution of soot size distribution in ethylene/air and ethylene/benzene/air flat flames was characterized by experimental measurements and model predictions of size and number concentration within the flames. Experimentally, a scanning mobility particle sizer was used to allow spatially resolved and online measurements of particle concentration and sizes in the nanometer-size range. The model couples a detailed kinetic scheme with a discrete-sectional approach to follow the transition from gas-phase to nascent particles and their coagulation to larger soot particles. The evolution of soot size distribution (experimental and modeled) in pure ethylene and ethylene flames doped with benzene showed a typical nucleation-sized (since particles do not actually nucleate in the classical sense particle inception is often used in place of nucleation) mode close to the burner surface, and a bimodal behavior at greater height above burner (HAB). However, major features were distinguished between the data sets. The growth of nucleation and agglomeration-sized particles was faster for ethylene/benzene/air flames, evidenced by the earlier presence of bimodality in these flames. The most significant changes in size distribution were attributed to an increase in benzene concentration in the initial fuel. However, these changes were more evident for high temperature flames. In agreement with the experimental data, the model also predicted the decrease of nucleation-sized particles in the postflame region for ethylene flames doped with benzene. This behavior was associated with the decrease of soot precursors after the main oxidation zone of the flames. (author)

  11. A general flamelet transformation useful for distinguishing between premixed and non-premixed modes of combustion

    SciTech Connect

    Knudsen, E.; Pitsch, H.

    2009-03-15

    The flame index was originally proposed by Yamashita et al. as a method of locally distinguishing between premixed and non-premixed combustion. Although this index has been applied both passively in the analysis of direct numerical simulation data, and actively using single step combustion models, certain limitations restrict its use in more detailed combustion models. In this work a general flamelet transformation that holds in the limits of both premixed and non-premixed combustion is developed. This transformation makes use of two statistically independent variables: a mixture fraction and a reaction progress parameter. The transformation is used to produce a model for distinguishing between premixed and non-premixed combustion regimes. The new model locally examines the term budget of the general flamelet transformation. The magnitudes of each of the terms in the budget are calculated and compared to the chemical source term. Determining whether a flame burns in a premixed or a non-premixed regime then amounts to determining which sets of these terms most significantly contribute to balancing the source term. The model is tested in a numerical simulation of a laminar triple flame, and is compared to a recent manifestation of the flame index approach. Additionally, the model is applied in a presumed probability density function (PDF) large eddy simulation (LES) of a lean premixed swirl burner. The model is used to locally select whether tabulated premixed or tabulated non-premixed chemistry should be referenced in the LES. Results from the LES are compared to experiments. (author)

  12. Pressure dependence of NO formation in laminar fuel-rich premixed CH{sub 4}/air flames

    SciTech Connect

    van Essen, V.M.; Sepman, A.V.; Mokhov, A.V.; Levinsky, H.B.

    2008-05-15

    Effects of pressure on NO formation in CH{sub 4}/air flames at a fixed equivalence ratio of 1.3 are investigated. The axial profiles of temperature, OH, CH, and NO mole fractions are measured using laser-induced fluorescence and compared with one-dimensional flame calculations. The measured and calculated temperature, CH, and NO profiles in free flames are observed to vary upon increasing the pressure from 40 to 75 Torr, following a scaling law derived for a chemical mechanism containing only second-order reactions. At pressures 300-760 Torr, the measurements and calculations in burner-stabilized flames show increasing flame temperature and NO mole fractions when the mass flux is increased linearly with pressure, while the CH profiles remain unchanged. The observed deviation from the scaling law in the temperature profiles arises from the increasing contribution of three-body reactions to the flame front propagation velocity, leading to a decrease in the degree of burner stabilization. The deviation from the pressure scaling law for the NO mole fractions is due to the temperature dependence of the rate coefficient for the reaction between CH and N{sub 2} and the fact that the temperature profiles themselves do not scale. In contrast, the surprisingly good scaling of the CH mole fractions with pressure indicates the dominant role of two-body reactions participating in the chain of chemical reactions leading to CH formation. The calculations using GRI-Mech 3.0 substantially overpredict (up to 50%) the measured nitric oxide concentrations for all pressures studied. The observed differences in the NO mole fraction may be addressed by improving the CH prediction. (author)

  13. FORMATION OF TRACE BYPRODUCTS IN THE PREMIXED FLAMES OF CH3CL/C2H4. (R825412)

    EPA Science Inventory

    The chemical structure of an atmospheric pressure, fuel-rich (equivalence
    ratio 3.06), flat flame of a chloromethane and ethylene
    (CH3Cl/C2H4 = 1.99) has been studied
    experimentally using both heated microprobe and cold trap samplin...

  14. Comparisons of Lagrangian and Eulerian PDF methods in simulations of non-premixed turbulent jet flames with moderate-to-strong turbulence-chemistry interactions

    NASA Astrophysics Data System (ADS)

    Jaishree, J.; Haworth, D. C.

    2012-06-01

    Transported probability density function (PDF) methods have been applied widely and effectively for modelling turbulent reacting flows. In most applications of PDF methods to date, Lagrangian particle Monte Carlo algorithms have been used to solve a modelled PDF transport equation. However, Lagrangian particle PDF methods are computationally intensive and are not readily integrated into conventional Eulerian computational fluid dynamics (CFD) codes. Eulerian field PDF methods have been proposed as an alternative. Here a systematic comparison is performed among three methods for solving the same underlying modelled composition PDF transport equation: a consistent hybrid Lagrangian particle/Eulerian mesh (LPEM) method, a stochastic Eulerian field (SEF) method and a deterministic Eulerian field method with a direct-quadrature-method-of-moments closure (a multi-environment PDF-MEPDF method). The comparisons have been made in simulations of a series of three non-premixed, piloted methane-air turbulent jet flames that exhibit progressively increasing levels of local extinction and turbulence-chemistry interactions: Sandia/TUD flames D, E and F. The three PDF methods have been implemented using the same underlying CFD solver, and results obtained using the three methods have been compared using (to the extent possible) equivalent physical models and numerical parameters. Reasonably converged mean and rms scalar profiles are obtained using 40 particles per cell for the LPEM method or 40 Eulerian fields for the SEF method. Results from these stochastic methods are compared with results obtained using two- and three-environment MEPDF methods. The relative advantages and disadvantages of each method in terms of accuracy and computational requirements are explored and identified. In general, the results obtained from the two stochastic methods (LPEM and SEF) are very similar, and are in closer agreement with experimental measurements than those obtained using the MEPDF method

  15. Numerical Study of Flame Stabilization Mechanism in a Premixed Burner with LES Non-adiabatic Flamelet Approach

    NASA Astrophysics Data System (ADS)

    Tang, Yihao; Hassanaly, Malik; Raman, Venkat

    2015-11-01

    In the development of highly efficient gas turbine combustion system, using high-hydrogen-content fuels is a new solution that limits pollutant emissions but also triggers flame stabilization issues. One promising concept to handle such instabilities within a large range of operating conditions is the FLOX® burner. A noticeable feature of the FLOX® burner is that it discharges high momentum jets without swirl, and flame stabilization is achieved in the shear layer around the jets. Experimental investigations have concluded that low velocity zones were absent and the flashback propensity was effectively decreased. It is proposed to study the stabilization mechanism to understand what physical phenomena are decisive in the process. In a preliminary numerical study, an adiabatic flamelet table was used along with LES simulations. Although the flow field's main features were captured, the simulation had issues in accurately predicting some important thermochemical quantities, including near wall quenching effects and OH mass fraction distribution. This work focuses on the effect of the adiabatic hypothesis on the flame stabilization mechanism. A non-adiabatic flamelet model is implemented and the impact on the stabilization mechanism is being quantified.

  16. Numerical studies of nitric oxide formation in nanosecond-pulsed discharge-stabilized flames of premixed methane/air.

    PubMed

    Bak, Moon Soo; Cappelli, Mark A

    2015-08-13

    A simulation is developed to investigate the kinetics of nitric oxide (NO) formation in premixed methane/air combustion stabilized by nanosecond-pulsed discharges. The simulation consists of two connected parts. The first part calculates the kinetics within the discharge while considering both plasma/combustion reactions and species diffusion, advection and thermal conduction to the surrounding flow. The second part calculates the kinetics of the overall flow after mixing the discharge flow with the surrounding flow to account for the effect that the discharge has on the overall kinetics. The simulation reveals that the discharge produces a significant amount of atomic oxygen (O) as a result of the high discharge temperature and dissociative quenching of excited state nitrogen by molecular oxygen. This atomic oxygen subsequently produces hydroxyl (OH) radicals. The fractions of these O and OH then undergo Zel'dovich reactions and are found to contribute to as much as 73% of the total NO that is produced. The post-discharge simulation shows that the NO survives within the flow once produced. PMID:26170428

  17. Triple flames and flame stabilization

    NASA Technical Reports Server (NTRS)

    Broadwell, James E.

    1994-01-01

    It is now well established that when turbulent jet flames are lifted, combustion begins, i.e., the flame is stabilized, at an axial station where the fuel and air are partially premixed. One might expect, therefore, that the beginning of the combustion zone would be a triple flame. Such flames have been described; however, other experiments provide data that are difficult to reconcile with the presence of triple flames. In particular, laser images of CH and OH, marking combustion zones, do not exhibit shapes typical of triple flames, and, more significantly, the lifted flame appears to have a propagation speed that is an order of magnitude higher than the laminar flame speed. The speed of triple flames studied thus far exceeds the laminar value by a factor less than two. The objective of the present task is the resolution of the apparent conflict between the experiments and the triple flame characteristics, and the clarification of the mechanisms controlling flame stability. Being investigated are the resolution achieved in the experiments, the flow field in the neighborhood of the stabilization point, propagation speeds of triple flames, laboratory flame unsteadiness, and the importance of flame ignition limits in the calculation of triple flames that resemble lifted flames.

  18. Characteristics of non-premixed oxygen-enhanced combustion: II. Flame structure effects on soot precursor kinetics resulting in soot-free flames

    SciTech Connect

    Skeen, S.A.; Axelbaum, R.L.; Yablonsky, G.

    2010-09-15

    A detailed computational study was performed to understand the effects of the flame structure on the formation and destruction of soot precursors during ethylene combustion. Using the USC Mech Version II mechanism the contributions of different pathways to the formation of benzene and phenyl were determined in a wide domain of Z{sub st} values via a reverse-pathway analysis. It was shown that for conventional ethylene-air flames two sequential reversible reactions play primary roles in the propargyl (C{sub 3}H{sub 3}) chemistry, namely (1) C{sub 2}H{sub 2}+CH{sub 3}= pC{sub 3} H{sub 4}+H, (2) pC{sub 3} H{sub 4}= C{sub 3} H{sub 3}+ H with the corresponding overall endothermic reaction of propargyl formation (3) C{sub 2} H{sub 2}+CH{sub 3}= C{sub 3} H{sub 3}+2H. The contributions of these reactions to propyne (pC{sub 3}H{sub 4}) and propargyl formation and propargyl self-combination leading to benzene and phenyl were studied as a function of physical position, temperature, Z{sub st}, and H concentration. In particular, the role of H radicals on soot precursor destruction was studied in detail. At low Z{sub st}, Reactions 1 and 2 contribute significantly to propyne and propargyl formation on the fuel side of the radical pool at temperatures greater than approx. 1600 K. At higher local temperatures near the radical pool where the concentration of H is significant, the reverse reactions begin to dominate resulting in soot precursor destruction. As Z{sub st} is increased, these regions merge and only net propargyl consumption is observed. Based on the equilibrium constant of Reaction 3, a Z{sub st} value was estimated above which the rate of propargyl formation as a soot precursor is greatly reduced (Z{sub st} = 0.3). This condition compares well with the experimental results for permanently blue counterflow flames in the literature. (author)

  19. Nitric Oxide and Oxygen Air-Contamination Effects on Extinction Limits of Non-Premixed Hydrocarbon-Air Flames for a HIFiRE Scramjet

    NASA Technical Reports Server (NTRS)

    Pellett, Gerald L.; Dawson, Lucy C.; Vaden, Sarah N.; Wilson, Lloyd G.

    2009-01-01

    Unique nitric oxide (NO) and oxygen air-contamination effects on the extinction Flame Strength (FS) of non-premixed hydrocarbon (HC) vs. air flames are characterized for 7 gaseous HCs, using a new idealized 9.3 mm straight-tube Opposed Jet Burner (OJB) at 1 atm. FS represents a laminar strain-induced extinction limit based on cross-section-average air jet velocity, Uair, that sustains combustion of a counter jet of gaseous fuel just before extinction. Besides ethane, propane, butane, and propylene, the HCs include ethylene, methane, and a 64 mole-% ethylene / 36 % methane mixture, the writer s previously recommended gaseous surrogate fuel for HIFiRE scramjet tests. The HC vs. clean air part of the work is an extension of a May 2008 JANNAF paper that characterized surrogates for the HIFiRE project that should mimic the flameholding of reformed (thermally- or catalytically-cracked) endothermic JP-like fuels. The new FS data for 7 HCs vs. clean air are thus consolidated with the previously validated data, normalized to absolute (local) axial-input strain rates, and co-plotted on a dual kinetically dominated reactivity scale. Excellent agreement with the prior data is obtained for all 7 fuels. Detailed comparisons are also made with recently published (Univ. Va) numerical results for ethylene extinction. A 2009-revised ethylene kinetic model (Univ. Southern Cal) led to predicted limits within approx. 5 % (compared to 45 %, earlier) of this writer s 2008 (and present) ethylene FSs, and also with recent independent data (Univ. Va) obtained on a new OJB system. These +/- 5 % agreements, and a hoped-for "near-identically-performing" reduced kinetics model, would greatly enhance the capability for accurate numerical simulations of surrogate HC flameholding in scramjets. The measured air-contamination effects on normalized FS extinction limits are projected to assess ongoing Arc-Heater-induced "facility test effects" of NO production (e.g., 3 mole-%) and resultant oxygen

  20. FLame

    1995-03-03

    FLAME is data processing software explicitly written to support the ACAP software of DSP Technologies, Inc., of Fremont, CA. ACAP acquires and processes in-cylinder pressure data for reciprocating engines. However, it also has the capability to acquire data for two Sandia-developed technologies, ionization-probe instrumented head gaskets and fiber-optic instrumented spark plugs. FLAME post processes measurements of flame arrival from data files aquired with ACAP. Flame arrival time is determined from analog ionization-probe or visible-emission signals.more » The resulting data files are integrated with the standard ACAP files, providing a common data base for engine development.« less

  1. A filtered tabulated chemistry model for LES of premixed combustion

    SciTech Connect

    Fiorina, B.; Auzillon, P.; Darabiha, N.; Gicquel, O.; Veynante, D.; Vicquelin, R.

    2010-03-15

    A new modeling strategy called F-TACLES (Filtered Tabulated Chemistry for Large Eddy Simulation) is developed to introduce tabulated chemistry methods in Large Eddy Simulation (LES) of turbulent premixed combustion. The objective is to recover the correct laminar flame propagation speed of the filtered flame front when subgrid scale turbulence vanishes as LES should tend toward Direct Numerical Simulation (DNS). The filtered flame structure is mapped using 1-D filtered laminar premixed flames. Closure of the filtered progress variable and the energy balance equations are carefully addressed in a fully compressible formulation. The methodology is first applied to 1-D filtered laminar flames, showing the ability of the model to recover the laminar flame speed and the correct chemical structure when the flame wrinkling is completely resolved. The model is then extended to turbulent combustion regimes by including subgrid scale wrinkling effects in the flame front propagation. Finally, preliminary tests of LES in a 3-D turbulent premixed flame are performed. (author)

  2. Oscillating combustion from a premix fuel nozzle

    SciTech Connect

    Richards, G.A.; Yip, M.J.

    1995-08-01

    Stringent emissions requirements for stationary gas turbines have produced new challenges in combustor design. In the past, very low NOx pollutant emissions have been achieved through various combustion modifications, such as steam or water injection, or post-combustion cleanup methods such as selective catalytic reduction (SCR). An emerging approach to NOx abatement is lean premix combustion. Lean premix combustion avoids the cost and operational problems associated with other NOx control methods. By premixing fuel and air at very low equivalence ratios, the high temperatures which produce NOx are avoided. The challenges of premix combustion include avoiding flashback, and ensuring adequate fuel/air premixing. In addition, the combustion must be stable. The combustor should not operate so close to extinction that a momentary upset will extinguish the flame (static stability), and the flame should not oscillate (dynamic stability). Oscillations are undesirable because the associated pressure fluctuations can shorten component lifetime. Unfortunately, experience has shown that premix fuel nozzles burning natural gas are susceptible to oscillations. Eliminating these oscillations can be a costly and time consuming part of new engine development. As part of the U.S. Department of Energy`s Advanced Turbine Systems Program, the Morgantown Energy Technology Center (METC) is investigating the issue of combustion oscillations produced by lean premix fuel nozzles. METC is evaluating various techniques to stabilize oscillating combustion in gas turbines. Tests results from a premix fuel nozzle using swirl stabilization and a pilot flame are reported here.

  3. On the thermodynamic properties of thermal plasma in the flame kernel of hydrocarbon/air premixed gases

    NASA Astrophysics Data System (ADS)

    Askari, Omid; Beretta, Gian Paolo; Eisazadeh-Far, Kian; Metghalchi, Hameed

    2016-07-01

    Thermodynamic properties of hydrocarbon/air plasma mixtures at ultra-high temperatures must be precisely calculated due to important influence on the flame kernel formation and propagation in combusting flows and spark discharge applications. A new algorithm based on the complete chemical equilibrium assumption is developed to calculate the ultra-high temperature plasma composition and thermodynamic properties, including enthalpy, entropy, Gibbs free energy, specific heat at constant pressure, specific heat ratio, speed of sound, mean molar mass, and degree of ionization. The method is applied to compute the thermodynamic properties of H2/air and CH4/air plasma mixtures for different temperatures (1000-100 000 K), different pressures (10-6-100 atm), and different fuel/air equivalence ratios within flammability limit. In calculating the individual thermodynamic properties of the atomic species needed to compute the complete equilibrium composition, the Debye-Huckel cutoff criterion has been used for terminating the series expression of the electronic partition function so as to capture the reduction of the ionization potential due to pressure and the intense connection between the electronic partition function and the thermodynamic properties of the atomic species and the number of energy levels taken into account. Partition functions have been calculated using tabulated data for available atomic energy levels. The Rydberg and Ritz extrapolation and interpolation laws have been used for energy levels which are not observed. The calculated plasma properties are then presented as functions of temperature, pressure and equivalence ratio, in terms of a new set of thermodynamically self-consistent correlations that are shown to provide very accurate fits suitable for efficient use in CFD simulations. Comparisons with existing data for air plasma show excellent agreement.

  4. Premixed direct injection nozzle

    DOEpatents

    Zuo, Baifang; Johnson, Thomas Edward; Lacy, Benjamin Paul; Ziminsky, Willy Steve

    2011-02-15

    An injection nozzle having a main body portion with an outer peripheral wall is disclosed. The nozzle includes a plurality of fuel/air mixing tubes disposed within the main body portion and a fuel flow passage fluidly connected to the plurality of fuel/air mixing tubes. Fuel and air are partially premixed inside the plurality of the tubes. A second body portion, having an outer peripheral wall extending between a first end and an opposite second end, is connected to the main body portion. The partially premixed fuel and air mixture from the first body portion gets further mixed inside the second body portion. The second body portion converges from the first end toward said second end. The second body portion also includes cooling passages that extend along all the walls around the second body to provide thermal damage resistance for occasional flame flash back into the second body.

  5. Combustor flame flashback

    NASA Technical Reports Server (NTRS)

    Proctor, M. P.; Tien, J. S.

    1985-01-01

    A stainless steel, two-dimensional (rectangular), center-dump, premixed-prevaporized combustor with quartz window sidewalls for visual access was designed, built, and used to study flashback. A parametric study revealed that the flashback equivalence ratio decreased slightly as the inlet air temperature increased. It also indicated that the average premixer velocity and premixer wall temperature were not governing parameters of flashback. The steady-state velocity balance concept as the flashback mechanism was not supported. From visual observation several stages of burning were identified. High speed photography verified upstream flame propagation with the leading edge of the flame front near the premixer wall. Combustion instabilities (spontaneous pressure oscillations) were discovered during combustion at the dump plane and during flashback. The pressure oscillation frequency ranged from 40 to 80 Hz. The peak-to-peak amplitude (up to 1.4 psi) increased as the fuel/air equivalence ratio was increased attaining a maximum value just before flashback. The amplitude suddenly decreased when the flame stabilized in the premixer. The pressure oscillations were large enough to cause a local flow reversal. A simple test using ceramic fiber tufts indicated flow reversals existed at the premixer exit during flickering. It is suspected that flashback occurs through the premixer wall boundary layer flow reversal caused by combustion instability. A theoretical analysis of periodic flow in the premixing channel has been made. The theory supports the flow reversal mechanism.

  6. LEM-CF Premixed Tool Kit

    SciTech Connect

    2015-01-19

    The purpose of LEM-CF Premixed Tool Kit is to process premixed flame simulation data from the LEM-CF solver (https://fileshare.craft-tech.com/clusters/view/lem-cf) into a large-eddy simulation (LES) subgrid model database. These databases may be used with a user-defined-function (UDF) that is included in the Tool Kit. The subgrid model UDF may be used with the ANSYS FLUENT flow solver or other commercial flow solvers.

  7. Atomic absorption spectroscopy with high temperature flames.

    PubMed

    Willis, J B

    1968-07-01

    An account is given of the history of the development of high temperature flames for the atomic absorption measurement of metals forming refractory oxides. The principles governing the design of premix burners for such flames, and the relative merits of different types of nebulizer burner systems are described. After a brief account of the structure and emission characteristics of the premixed oxygen-acetylene and nitrous oxide-acetylene flames, the scope and limitations of the latter flame in chemical analysis are discussed.

  8. A premixed hydrogen/oxygen catalytic igniter

    NASA Technical Reports Server (NTRS)

    Green, James M.

    1989-01-01

    The catalytic ignition of hydrogen and oxygen propellants was studied using a premixing hydrogen/oxygen injector. The premixed injector was designed to eliminate problems associated with catalytic ignition caused by poor propellant mixing in the catalyst bed. Mixture ratio, mass flow rate, and propellant inlet temperature were varied parametrically in testing, and a pulse mode life test of the igniter was conducted. The results of the tests showed that the premixed injector eliminated flame flashback in the reactor and increased the life of the igniter significantly. The results of the experimental program and a comparison with data collected in a previous program are given.

  9. Dynamics and structure of stretched flames

    SciTech Connect

    Law, C.K.

    1993-12-01

    This program aims to gain fundamental understanding on the structure, geometry, and dynamics of laminar premixed flames, and relate these understanding to the practical issues of flame extinction and stabilization. The underlying fundamental interest here is the recent recognition that the response of premixed flames can be profoundly affected by flame stretch, as manifested by flow nonuniformity, flame curvature, and flame/flow unsteadiness. As such, many of the existing understanding on the behavior of premixed flames need to be qualitatively revised. The research program consists of three major thrusts: (1) detailed experimental and computational mapping of the structure of aerodynamically-strained planar flames, with emphasis on the effects of heat loss, nonequidiffusion, and finite residence time on the flame thickness, extent of incomplete reaction, and the state of extinction. (2) Analytical study of the geometry and dynamics of stretch-affected wrinkled flame sheets in simple configurations, as exemplified by the Bunsen flame and the spatially-periodic flame, with emphasis on the effects of nonlinear stretch, the phenomena of flame cusping, smoothing, and tip opening, and their implications on the structure and burning rate of turbulent flames. (3) Stabilization and blowoff of two-dimensional inverted premixed and stabilization and determining the criteria governing flame blowoff. The research is synergistically conducted through the use of laser-based diagnostics, computational simulation of the flame structure with detailed chemistry and transport, and mathematical analysis of the flame dynamics.

  10. Detailed modeling and laser-induced fluorescence imaging of nitric oxide in a NH(i)-seeded non-premixed methane/air flame

    SciTech Connect

    Bell, John B.; Day, Marcus S.; Grcar, Joseph F.; Bessler, Wolfgang G.; Schulz, Christof; Glarborg, Peter; Jensen, Anker D.

    2001-12-14

    In this paper we study the formation of NO in laminar, nitrogen diluted methane diffusion flames that are seeded with ammonia in the fuel stream. We have performed numerical simulations with detailed chemistry as well as laser-induced fluorescence imaging measurements for a range of ammonia injection rates. For comparison with the experimental data, synthetic LIF images are calculated based on the numerical data accounting for temperature and fluorescence quenching effects. We demonstrate good agreement between measurements and computations. The LIF corrections inferred from the simulation are then used to calculate absolute NO mole fractions from the measured signal.The NO formation in both doped and undoped flames occurs in the flame sheet. In the undoped flame, four different mechanisms including thermal and prompt NO appear to contribute to NO formation. As the NH3 seeding level increases, fuel-NO becomes the dominant mechanism and N2 shifts from being a net reactant to being a net product. Nitric oxide in the undoped flame as well as in the core region of the doped flames are underpredicted by the model; we attribute this mainly to inaccuracies in the NO recycling chemistry on the fuel-rich side of the flame sheet.

  11. Premixed direct injection disk

    SciTech Connect

    York, William David; Ziminsky, Willy Steve; Johnson, Thomas Edward; Lacy, Benjamin; Zuo, Baifang; Uhm, Jong Ho

    2013-04-23

    A fuel/air mixing disk for use in a fuel/air mixing combustor assembly is provided. The disk includes a first face, a second face, and at least one fuel plenum disposed therebetween. A plurality of fuel/air mixing tubes extend through the pre-mixing disk, each mixing tube including an outer tube wall extending axially along a tube axis and in fluid communication with the at least one fuel plenum. At least a portion of the plurality of fuel/air mixing tubes further includes at least one fuel injection hole have a fuel injection hole diameter extending through said outer tube wall, the fuel injection hole having an injection angle relative to the tube axis. The invention provides good fuel air mixing with low combustion generated NOx and low flow pressure loss translating to a high gas turbine efficiency, that is durable, and resistant to flame holding and flash back.

  12. Numerical simulation of premixed turbulent methane combustion

    SciTech Connect

    Bell, John B.; Day, Marcus S.; Grcar, Joseph F.

    2001-12-14

    In this paper we study the behavior of a premixed turbulent methane flame in three dimensions using numerical simulation. The simulations are performed using an adaptive time-dependent low Mach number combustion algorithm based on a second-order projection formulation that conserves both species mass and total enthalpy. The species and enthalpy equations are treated using an operator-split approach that incorporates stiff integration techniques for modeling detailed chemical kinetics. The methodology also incorporates a mixture model for differential diffusion. For the simulations presented here, methane chemistry and transport are modeled using the DRM-19 (19-species, 84-reaction) mechanism derived from the GRIMech-1.2 mechanism along with its associated thermodynamics and transport databases. We consider a lean flame with equivalence ratio 0.8 for two different levels of turbulent intensity. For each case we examine the basic structure of the flame including turbulent flame speed and flame surface area. The results indicate that flame wrinkling is the dominant factor leading to the increased turbulent flame speed. Joint probability distributions are computed to establish a correlation between heat release and curvature. We also investigate the effect of turbulent flame interaction on the flame chemistry. We identify specific flame intermediates that are sensitive to turbulence and explore various correlations between these species and local flame curvature. We identify different mechanisms by which turbulence modulates the chemistry of the flame.

  13. Aerodynamics of Laminar Flames

    NASA Astrophysics Data System (ADS)

    Law, Chung K.

    2000-11-01

    The presentation will review recent advances in the understanding of the structure, dynamics, and geometry of stretched, nonequidiffusive, laminar premixed flames, as exemplified by the unsteady propagation of wrinkled flames in nonuniform flow fields. It is first shown that by considering the effects of aerodynamic stretch on the flame structure, and by allowing for mixture nonequidiffusion, the flame responses, especially the flame propagation speed, can be quantitatively as well as qualitatively modified from the idealized planar limit. Subsequently, by treating the flame as a level surface propagating with the stretch-affected flame speed, problems of increasing complexity are presented to illustrate various features of flame propagation. The illustration first treats the flame as a structureless surface propagating into a constant-density combustible with a constant velocity * the laminar flame speed, and demonstrates the phenomena of cusp formation and volumetric burning rate augmentation through flame wrinkling. By using the stretch-affected flame speed, we then describe the phenomena of cusp broadening as well as tip opening of the Bunsen flame. Finally, by allowing for the density jump across the flame surface, a unified dispersion relation is derived for the intrinsic hydrodynamic, body-force, and nonequidiffusive modes of flame

  14. Effect of finite-rate chemistry and unequal Schmidt numbers on turbulent non-premixed flames modeled with single-step chemistry

    NASA Technical Reports Server (NTRS)

    Chen, J. H.; Mahalingam, S.; Puri, I. K.; Vervisch, L.

    1992-01-01

    The interaction between a quasi-laminar flame and a turbulent flowfield is investigated through direct numerical simulations (DNS) of reacting flow in two- and three-dimensional domains. Effects due to finite-rate chemistry are studied using a single step global reaction A (fuel) + B (oxidizer) yields P (product), and by varying a global Damkoehler number, as a result of which the turbulence-chemistry interaction in the flame is found to generate a wide variety of conditions, ranging from near-equilibrium to near-extinction. Differential diffusion effects are studied by changing the Schmidt number of one reactive species to one-half. It is observed that laminar flamelet response is followed within the turbulent flowfield, except in regions where transient effects seem to dominate.

  15. Large-Eddy Simulation of Premixed and Partially Premixed Turbulent Combustion Using a Level Set Method

    NASA Astrophysics Data System (ADS)

    Duchamp de Lageneste, Laurent; Pitsch, Heinz

    2001-11-01

    Level-set methods (G-equation) have been recently used in the context of RANS to model turbulent premixed (Hermann 2000) or partially premixed (Chen 1999) combustion. By directly taking into account unsteady effects, LES can be expected to improve predictions over RANS. Since the reaction zone thickness of premixed flames in technical devices is usually much smaller than the LES grid spacing, chemical reactions completely occur on the sub-grid scales and hence have to be modeled entirely. In the level-set methodology, the flame front is represented by an arbitrary iso-surface G0 of a scalar field G whose evolution is described by the so-called G-equation. This equation is only valid at G=G_0, and hence decoupled from other G levels. Heat release is then modeled using a flamelet approach in which temperature is determined as a function of G and the mixture-fraction Z. In the present study, the proposed approach has been formulated for LES and validated using data from a turbulent Bunsen burner experiment (Chen, Peters 1996). Simulation of an experimental Lean Premixed Prevapourised (LPP) dump combustor (Besson, Bruel 1999, 2000) under different premixed or partially premixed conditions will also be presented.

  16. Chaos in an imperfectly premixed model combustor

    SciTech Connect

    Kabiraj, Lipika Saurabh, Aditya; Paschereit, Christian O.; Karimi, Nader; Sailor, Anna; Mastorakos, Epaminondas; Dowling, Ann P.

    2015-02-15

    This article reports nonlinear bifurcations observed in a laboratory scale, turbulent combustor operating under imperfectly premixed mode with global equivalence ratio as the control parameter. The results indicate that the dynamics of thermoacoustic instability correspond to quasi-periodic bifurcation to low-dimensional, deterministic chaos, a route that is common to a variety of dissipative nonlinear systems. The results support the recent identification of bifurcation scenarios in a laminar premixed flame combustor (Kabiraj et al., Chaos: Interdiscip. J. Nonlinear Sci. 22, 023129 (2012)) and extend the observation to a practically relevant combustor configuration.

  17. Studies of Flame Structure in Microgravity

    NASA Technical Reports Server (NTRS)

    Law, C. K.; Sung, C. J.; Zhu, D. L.

    1997-01-01

    The present research endeavor is concerned with gaining fundamental understanding of the configuration, structure, and dynamics of laminar premixed and diffusion flames under conditions of negligible effects of gravity. Of particular interest is the potential to establish and hence study the properties of spherically- and cylindrically-symmetric flames and their response to external forces not related to gravity. For example, in an earlier experimental study of the burner-stabilized cylindrical premixed flames, the possibility of flame stabilization through flow divergence was established, while the resulting one-dimensional, adiabatic, stretchless flame also allowed an accurate means of determining the laminar flame speeds of combustible mixtures. We have recently extended our studies of the flame structure in microgravity along the following directions: (1) Analysis of the dynamics of spherical premixed flames; (2) Analysis of the spreading of cylindrical diffusion flames; (3) Experimental observation of an interesting dual luminous zone structure of a steady-state, microbuoyancy, spherical diffusion flame of air burning in a hydrogen/methane mixture environment, and its subsequent quantification through computational simulation with detailed chemistry and transport; (4) Experimental quantification of the unsteady growth of a spherical diffusion flame; and (5) Computational simulation of stretched, diffusionally-imbalanced premixed flames near and beyond the conventional limits of flammability, and the substantiation of the concept of extended limits of flammability. Motivation and results of these investigations are individually discussed.

  18. Oscillatory Extinction Of Spherical Diffusion Flames

    NASA Technical Reports Server (NTRS)

    Law, C. K.; Yoo, S. W.; Christianson, E. W.

    2003-01-01

    Since extinction has been observed in an oscillatory manner in Le greater than 1 premixed flames, it is not unreasonable to expect that extinction could occur in an unsteady manner for diffusion flames. Indeed, near-limit oscillations have been observed experimentally under microgravity conditions for both candle flames and droplet flames. Furthermore, the analysis of Cheatham and Matalon on the unsteady behavior of diffusion flames with heat loss, identified an oscillatory regime which could be triggered by either a sufficiently large Lewis number (even without heat loss) or an appreciable heat loss (even for Le=1). In light of these recent understanding, the present investigation aims to provide a well-controlled experiment that can unambiguously demonstrate the oscillation of diffusion flames near both the transport- and radiation-induced limits. That is, since candle and jet flames are stabilized through flame segments that are fundamentally premixed in nature, and since premixed flames are prone to oscillate, there is the possibility that the observed oscillation of these bulk diffusion flames could be triggered and sustained by the oscillation of the premixed flame segments. Concerning the observed oscillatory droplet extinction, it is well-known that gas-phase oscillation in heterogeneous burning can be induced by and is thereby coupled with condensed-phase unsteadiness. Consequently, a convincing experiment on diffusion flame oscillation must exclude any ingredients of premixed flames and other sources that may either oscillate themselves or promote the oscillation of the diffusion flame. The present experiment on burner-generated spherical flames with a constant reactant supply endeavored to accomplish this goal. The results are further compared with those from computational simulation for further understanding and quantification of the flame dynamics and extinction.

  19. Lagrangian formulation of turbulent premixed combustion.

    PubMed

    Pagnini, Gianni; Bonomi, Ernesto

    2011-07-22

    The lagrangian point of view is adopted to study turbulent premixed combustion. The evolution of the volume fraction of combustion products is established by the Reynolds transport theorem. It emerges that the burned-mass fraction is led by the turbulent particle motion, by the flame front velocity, and by the mean curvature of the flame front. A physical requirement connecting particle turbulent dispersion and flame front velocity is obtained from equating the expansion rates of the flame front progression and of the unburned particles spread. The resulting description compares favorably with experimental data. In the case of a zero-curvature flame, with a non-markovian parabolic model for turbulent dispersion, the formulation yields the Zimont equation extended to all elapsed times and fully determined by turbulence characteristics. The exact solution of the extended Zimont equation is calculated and analyzed to bring out different regimes.

  20. Hydrodynamic instability and shear layer effects in turbulent premixed combustion

    NASA Astrophysics Data System (ADS)

    Schlimpert, S.; Feldhusen, A.; Grimmen, J. H.; Roidl, B.; Meinke, M.; Schröder, W.

    2016-01-01

    A turbulent premixed plane jet flame is analyzed by large-eddy simulations. The analysis shows that the flame front wrinkling is strongly influenced by the shear layer effect when the gas expansion effects are small leading to larger flame front amplitudes at the flame base than at high gas expansion ratios. However, the hydrodynamic instability effect induces a continuously increasing flame front amplitude which yields an enhanced flame pocket generation at the flame tip. Both phenomena influence the magnitude of the turbulent burning area and burning area rate response through the flame front deflections which are determined by the contribution coefficient. This coefficient represents the mutual interaction between the flame and the flow. At low gas expansion ratios, the total heat release rate spectra of the turbulent flame are wider in terms of dominant modes at Strouhal numbers which are linked to the mean flame height oscillations. Thus, at low gas expansion ratios, the vortex-flame interaction is less damped by the flame in the sense that vortices can perturb the flame front stronger. The total heat release rate trend of St-2.2 previously found for a round jet flame is also determined for the current slot jet at realistic gas expansion ratios indicating a general tendency to transfer energy from large to small flame structures. At high gas expansion ratios, an increasing Markstein length leads to an energy transfer between neighboring dominant modes in the low frequency range 1 < St < 10 and the burning area rate response becomes more important for the total heat release rate spectra of the turbulent slot flames which agrees with recent findings for a laminar premixed plane flame.

  1. The stabilization of a methane-air edge flame within a mixing layer in a narrow channel

    SciTech Connect

    Lee, Min Jung; Kim, Nam Il

    2010-01-15

    The flame stabilization mechanism of a methane-air edge flame formulated in a narrow channel was experimentally investigated and compared with a simple analytical model. Non-premixed flames were classified into premixed flame modes and edge flame modes. The correlation between the propagation velocity and the fuel concentration gradient in a narrow channel was investigated and the applicability of ordinary edge-flame theory was appraised. (author)

  2. Multiple tube premixing device

    DOEpatents

    Uhm, Jong Ho; Naidu, Balachandar; Ziminksy, Willy Steve; Kraemer, Gilbert Otto; Yilmaz, Ertan; Lacy, Benjamin; Stevenson, Christian; Felling, David

    2013-08-13

    The present application provides a premixer for a combustor. The premixer may include a fuel plenum with a number of fuel tubes and a burner tube with a number of air tubes. The fuel tubes extend about the air tubes.

  3. Multiple tube premixing device

    DOEpatents

    Uhm, Jong Ho; Varatharajan, Balachandar; Ziminsky, Willy Steve; Kraemer, Gilbert Otto; Yilmaz, Ertan; Lacy, Benjamin; Stevenson, Christian; Felling, David

    2012-12-11

    The present application provides a premixer for a combustor. The premixer may include a fuel plenum with a number of fuel tubes and a burner tube with a number of air tubes. The fuel tubes extend about the air tubes.

  4. Quantitative measurement of hydroxyl radical (OH) concentration in premixed flat flame by combining laser-induced fluorescence and direct absorption spectroscopy

    NASA Astrophysics Data System (ADS)

    Chen, Shuang; Su, Tie; Li, Zhong-Shan; Bai, Han-Chen; Yan, Bo; Yang, Fu-Rong

    2016-10-01

    An accurate and reasonable technique combining direct absorption spectroscopy and laser-induced fluorescence (LIF) methods is developed to quantitatively measure the concentrations of hydroxyl in CH4/air flat laminar flame. In our approach, particular attention is paid to the linear laser-induced fluorescence and absorption processes, and experimental details as well. Through measuring the temperature, LIF signal distribution and integrated absorption, spatially absolute OH concentrations profiles are successfully resolved. These experimental results are then compared with the numerical simulation. It is proved that the good quality of the results implies that this method is suitable for calibrating the OH-PLIF measurement in a practical combustor. Project supported by the National Natural Science Foundation of China (Grant No. 11272338), the Science and Technology on Scramjet Key Laboratory Funding, China (Grant No. STSKFKT 2013004), and the China Scholarship Council.

  5. Flame-acoustic coupling of combustion instability in a non-premixed backward-facing step combustor: the role of acoustic-Reynolds stress

    NASA Astrophysics Data System (ADS)

    Kannan, Ashwin; Chellappan, Balaji; Chakravarthy, Satyanarayanan

    2016-07-01

    Combustion instability in a laboratory scale backward-facing step combustor is numerically investigated by carrying out an acoustically coupled incompressible large eddy simulation of turbulent reacting flow for various Reynolds numbers with fuel injection at the step. The problem is mathematically formulated as a decomposition of the full compressible Navier-Stokes equations using multi-scale analysis by recognising the small length scale and large time scale of the flow field relative to a longitudinal mode acoustic field for low mean Mach numbers. The equations are decomposed into those for an incompressible flow with temperature-dependent density to zeroth order and linearised Euler equations for acoustics as a first order compressibility correction. Explicit coupling terms between the two equation sets are identified to be the flow dilatation as a source of acoustic energy and the acoustic Reynolds stress (ARS) as a source of flow momentum. The numerical simulations are able to capture the experimentally observed flow-acoustic lock-on that signifies the onset of combustion instability, marked by a shift in the dominant frequency from an acoustic to a hydrodynamic mode and accompanied by a nonlinear variation of pressure amplitude. Attention is devoted to flow conditions at two Reynolds numbers before and after lock-on to show that, after lock-on, the ARS causes large-scale vortical rollup resulting in the evolution of a compact flame. As compared to acoustically uncoupled simulations at these Reynolds numbers that show an elongated flame with no significant roll up and disturbance in the upstream flow field, the ARS is seen to alter the shear layer dynamics by affecting the flow field upstream of the step as well, when acoustically coupled.

  6. Mechanisms and enhancement of flame stabilization

    SciTech Connect

    Law, C.K.

    1993-01-01

    During the reporting period, useful contributions have been made in understanding the structure of laminar premixed and diffusion flames, with emphasis on the influence of aerodynamics and chemical kinetics. These contributions include (1) derivation of the missing closure condition for the activation energy asymptotic analysis of premixed flames, (2) identification of a dual extinction mode for radiation-affected flames, (3) formulation of a unified theory of fundamental flammability limits, and (4) demonstration that flame stabilization can be achieved in the absence of heat loss. These investigations have been conducted via experimental, analytical and computational approaches, with strong coupling between the individual components.

  7. Premixed Combustion Model for Boron Clouds

    NASA Astrophysics Data System (ADS)

    Wang, Mengze; Han, Wang; Chen, Zheng

    2015-11-01

    Boron particle is an ideal additive in solid propellants and fuels due to its very high volumetric heat release. In this study, a premixed combustion model for boron clouds is developed based on a previous combustion model for single boron particle. The flame structure is assumed to be composed of three zones: the preheat zone, the ignition zone, and the reaction zone, and analytical solutions are derived from the governing equations. Consequently the influence of the boron clouds' physical properties on the flame propagation process is investigated.

  8. Simulation of lean premixed turbulent combustion

    SciTech Connect

    Bell, John B.; Day, Marcus S.; Almgren, Ann S.; Lijewski, MichaelJ.; Rendleman, Charles A.; Cheng, Robert K.; Shepherd, Ian G.

    2006-06-25

    There is considerable technological interest in developingnew fuel-flexible combustion systems that can burn fuels such ashydrogenor syngas. Lean premixed systems have the potential to burn thesetypes of fuels with high efficiency and low NOx emissions due to reducedburnt gas temperatures. Although traditional scientific approaches basedon theory and laboratory experiment have played essential roles indeveloping our current understanding of premixed combustion, they areunable to meet the challenges of designing fuel-flexible lean premixedcombustion devices. Computation, with itsability to deal with complexityand its unlimited access to data, hasthe potential for addressing thesechallenges. Realizing this potential requires the ability to perform highfidelity simulations of turbulent lean premixed flames under realisticconditions. In this paper, we examine the specialized mathematicalstructure of these combustion problems and discuss simulation approachesthat exploit this structure. Using these ideas we can dramatically reducecomputational cost, making it possible to perform high-fidelitysimulations of realistic flames. We illustrate this methodology byconsidering ultra-lean hydrogen flames and discuss how this type ofsimulation is changing the way researchers study combustion.

  9. Pdf modeling for premixed turbulent combustion based on the properties of iso-concentration surfaces

    NASA Technical Reports Server (NTRS)

    Vervisch, L.; Kollmann, W.; Bray, K. N. C.; Mantel, T.

    1994-01-01

    In premixed turbulent flames the presence of intense mixing zones located in front of and behind the flame surface leads to a requirement to study the behavior of iso-concentration surfaces defined for all values of the progress variable (equal to unity in burnt gases and to zero in fresh mixtures). To support this study, some theoretical and mathematical tools devoted to level surfaces are first developed. Then a database of direct numerical simulations of turbulent premixed flames is generated and used to investigate the internal structure of the flame brush, and a new pdf model based on the properties of iso-surfaces is proposed.

  10. Spectral kinetic energy transfer in turbulent premixed reacting flows.

    PubMed

    Towery, C A Z; Poludnenko, A Y; Urzay, J; O'Brien, J; Ihme, M; Hamlington, P E

    2016-05-01

    Spectral kinetic energy transfer by advective processes in turbulent premixed reacting flows is examined using data from a direct numerical simulation of a statistically planar turbulent premixed flame. Two-dimensional turbulence kinetic-energy spectra conditioned on the planar-averaged reactant mass fraction are computed through the flame brush and variations in the spectra are connected to terms in the spectral kinetic energy transport equation. Conditional kinetic energy spectra show that turbulent small-scale motions are suppressed in the burnt combustion products, while the energy content of the mean flow increases. An analysis of spectral kinetic energy transfer further indicates that, contrary to the net down-scale transfer of energy found in the unburnt reactants, advective processes transfer energy from small to large scales in the flame brush close to the products. Triadic interactions calculated through the flame brush show that this net up-scale transfer of energy occurs primarily at spatial scales near the laminar flame thermal width. The present results thus indicate that advective processes in premixed reacting flows contribute to energy backscatter near the scale of the flame.

  11. Spectral kinetic energy transfer in turbulent premixed reacting flows

    NASA Astrophysics Data System (ADS)

    Towery, C. A. Z.; Poludnenko, A. Y.; Urzay, J.; O'Brien, J.; Ihme, M.; Hamlington, P. E.

    2016-05-01

    Spectral kinetic energy transfer by advective processes in turbulent premixed reacting flows is examined using data from a direct numerical simulation of a statistically planar turbulent premixed flame. Two-dimensional turbulence kinetic-energy spectra conditioned on the planar-averaged reactant mass fraction are computed through the flame brush and variations in the spectra are connected to terms in the spectral kinetic energy transport equation. Conditional kinetic energy spectra show that turbulent small-scale motions are suppressed in the burnt combustion products, while the energy content of the mean flow increases. An analysis of spectral kinetic energy transfer further indicates that, contrary to the net down-scale transfer of energy found in the unburnt reactants, advective processes transfer energy from small to large scales in the flame brush close to the products. Triadic interactions calculated through the flame brush show that this net up-scale transfer of energy occurs primarily at spatial scales near the laminar flame thermal width. The present results thus indicate that advective processes in premixed reacting flows contribute to energy backscatter near the scale of the flame.

  12. Stretching and quenching of flamelets in premixed turbulent combustion

    SciTech Connect

    Meneveau, C. ); Poinsot, T. )

    1991-09-01

    This paper reports on the stretch rate of flamelets in premixed turbulent combustion which is computed using detailed numerical simulations of vortex-flame interactions and a model for intermittent turbulence taking into account all possible turbulence scales acting on the flame front. Simulations of interactions between isolated vortices and a laminar flame front are used to obtain a relation between the characteristics of a given vortex and the actual flame stretch generated by this structure. Quenching conditions and quenching times are also given by these simulations. A net rate of stretch is then defined in the case of a complete turbulent flow field as the difference between the total rate of flame stretch and the quenching rate due to scales that have a high enough energy and a long enough lifetime to quench locally the flame front. The net rate of stretch is computed for a variety of parameters of interest in practical applications. It is a function of the large-scale turbulence parameters and the laminar flame speed and flame thickness and may be used as an input in most flamelet models for premixed turbulent combustion.

  13. Large eddy simulation of premixed and non-premixed combustion in a Stagnation Point Reverse Flow combustor

    NASA Astrophysics Data System (ADS)

    Undapalli, Satish

    A new combustor referred to as Stagnation Point Reverse Flow (SPRF) combustor has been developed at Georgia Tech to meet the increasingly stringent emission regulations. The combustor incorporates a novel design to meet the conflicting requirements of low pollution and high stability in both premixed and non-premixed modes. The objective of this thesis work is to perform Large Eddy Simulations (LES) on this lab-scale combustor and elucidate the underlying physics that has resulted in its excellent performance. To achieve this, numerical simulations have been performed in both the premixed and non-premixed combustion modes, and velocity field, species field, entrainment characteristics, flame structure, emissions, and mixing characteristics have been analyzed. Simulations have been carried out first for a non-reactive case to resolve relevant fluid mechanics without heat release by the computational grid. The computed mean and RMS quantities in the non-reacting case compared well with the experimental data. Next, the simulations were extended for the premixed reactive case by employing different sub-grid scale combustion chemistry closures: Eddy Break Up (EBU), Artificially Thickened Flame (TF) and Linear Eddy Mixing (LEM) models. Results from the EBU and TF models exhibit reasonable agreement with the experimental velocity field. However, the computed thermal and species fields have noticeable discrepancies. Only LEM with LES (LEMLES), which is an advanced scalar approach, has been able to accurately predict both the velocity and species fields. Scalar mixing plays an important role in combustion, and this is solved directly at the sub-grid scales in LEM. As a result, LEM accurately predicts the scalar fields. Due to the two way coupling between the super-grid and sub-grid quantities, the velocity predictions also compare very well with the experiments. In other approaches, the sub-grid effects have been either modeled using conventional approaches (EBU) or need

  14. Diffusion Flame Stabilization

    NASA Technical Reports Server (NTRS)

    Takahashi, Fumiaki; Katta, V. R.

    2006-01-01

    Diffusion flames are commonly used for industrial burners in furnaces and flares. Oxygen/fuel burners are usually diffusion burners, primarily for safety reasons, to prevent flashback and explosion in a potentially dangerous system. Furthermore, in most fires, condensed materials pyrolyze, vaporize, and burn in air as diffusion flames. As a result of the interaction of a diffusion flame with burner or condensed-fuel surfaces, a quenched space is formed, thus leaving a diffusion flame edge, which plays an important role in flame holding in combustion systems and fire spread through condensed fuels. Despite a long history of jet diffusion flame studies, lifting/blowoff mechanisms have not yet been fully understood, compared to those of premixed flames. In this study, the structure and stability of diffusion flames of gaseous hydrocarbon fuels in coflowing air at normal earth gravity have been investigated experimentally and computationally. Measurements of the critical mean jet velocity (U(sub jc)) of methane, ethane, or propane at lifting or blowoff were made as a function of the coflowing air velocity (U(sub a)) using a tube burner (i.d.: 2.87 mm). By using a computational fluid dynamics code with 33 species and 112 elementary reaction steps, the internal chemical-kinetic structures of the stabilizing region of methane and propane flames were investigated. A peak reactivity spot, i.e., reaction kernel, is formed in the flame stabilizing region due to back-diffusion of heat and radical species against an oxygen-rich incoming flow, thus holding the trailing diffusion flame. The simulated flame base moved downstream under flow conditions close to the measured stability limit.

  15. Diffusion Flame Stabilization

    NASA Technical Reports Server (NTRS)

    Takahashi, Fumiaki; Katta, Viswanath R.

    2007-01-01

    Diffusion flames are commonly used for industrial burners in furnaces and flares. Oxygen/fuel burners are usually diffusion burners, primarily for safety reasons, to prevent flashback and explosion in a potentially dangerous system. Furthermore, in most fires, condensed materials pyrolyze, vaporize, and burn in air as diffusion flames. As a result of the interaction of a diffusion flame with burner or condensed-fuel surfaces, a quenched space is formed, thus leaving a diffusion flame edge, which plays an important role in flame holding in combustion systems and fire spread through condensed fuels. Despite a long history of jet diffusion flame studies, lifting/blowoff mechanisms have not yet been fully understood, compared to those of premixed flames. In this study, the structure and stability of diffusion flames of gaseous hydrocarbon fuels in coflowing air at normal earth gravity have been investigated experimentally and computationally. Measurements of the critical mean jet velocity (U(sub jc)) of methane, ethane, or propane at lifting or blowoff were made as a function of the coflowing air velocity (U(sub a)) using a tube burner (i.d.: 2.87 mm) (Fig. 1, left). By using a computational fluid dynamics code with 33 species and 112 elementary reaction steps, the internal chemical-kinetic structures of the stabilizing region of methane and propane flames were investigated (Fig. 1, right). A peak reactivity spot, i.e., reaction kernel, is formed in the flame stabilizing region due to back-diffusion of heat and radical species against an oxygen-rich incoming flow, thus holding the trailing diffusion flame. The simulated flame base moved downstream under flow conditions close to the measured stability limit.

  16. Computational Studies of Flame Structures

    NASA Astrophysics Data System (ADS)

    Amin, Vaishali

    This thesis is concerned with computational studies of laminar flame structures using detailed and skeletal chemical kinetic mechanisms. Elementary reactions in these mechanisms control the observable combustion properties such as flame speed, autoignition temperature, ignition delay time, and extinction characteristics in nonpremixed and premixed flame phenomena. First part of thesis deals with computational investigations of influence of carbon monoxide and hydrogen addition on methane flames stabilized in counterflow configuration. Computations were performed employing detailed chemical kinetic mechanism---the San Diego mechanism. In case of nonpremixed flames, effect of carbon xvi monoxide addition on structure and critical condition of extinction were examined. Differences between addition on fuel and oxidizer sides were investigated and plausible explanation given for the differences. For premixed flames, effect of addition of hydrogen and carbon monoxide to reactant mixture was studied. Critical conditions of extinction were predicted using computations for various compositions. Rates of production and consumption of various species were calculated and flame structure was analyzed for nonpremixed and premixed flames. It was found that moderate amount of carbon monoxide addition to methane enhances flame reactivity. However, with large amount of carbon monoxide addition, additive chemistry dominates. Addition of increasing amounts of hydrogen in premixed reactant stream enhances methane flame reactivity. In second part of thesis, kinetic modeling was performed to elucidate the structure and mechanism of extinction and autoignition of nonpremixed toluene flames in counterflow configuration. Computations were performed using detailed chemistry to determine flame structure and to obtain values for critical conditions of extinction and autoignition. Sensitivity analysis of rate parameters, reaction pathway analysis, and spatial reaction rate profiles were used to

  17. Gas turbine premixing systems

    DOEpatents

    Kraemer, Gilbert Otto; Varatharajan, Balachandar; Evulet, Andrei Tristan; Yilmaz, Ertan; Lacy, Benjamin Paul

    2013-12-31

    Methods and systems are provided for premixing combustion fuel and air within gas turbines. In one embodiment, a combustor includes an upstream mixing panel configured to direct compressed air and combustion fuel through premixing zone to form a fuel-air mixture. The combustor includes a downstream mixing panel configured to mix additional combustion fuel with the fule-air mixture to form a combustion mixture.

  18. Combustion-acoustic stability analysis for premixed gas turbine combustors

    NASA Technical Reports Server (NTRS)

    Darling, Douglas; Radhakrishnan, Krishnan; Oyediran, Ayo; Cowan, Lizabeth

    1995-01-01

    Lean, prevaporized, premixed combustors are susceptible to combustion-acoustic instabilities. A model was developed to predict eigenvalues of axial modes for combustion-acoustic interactions in a premixed combustor. This work extends previous work by including variable area and detailed chemical kinetics mechanisms, using the code LSENS. Thus the acoustic equations could be integrated through the flame zone. Linear perturbations were made of the continuity, momentum, energy, chemical species, and state equations. The qualitative accuracy of our approach was checked by examining its predictions for various unsteady heat release rate models. Perturbations in fuel flow rate are currently being added to the model.

  19. Visible emission of hydrogen flames

    SciTech Connect

    Schefer, R.W.; Kulatilaka, W.D.; Patterson, B.D.; Settersten, T.B.

    2009-06-15

    The common misconception that hydrogen flames are not visible is examined. Examples are presented of clearly visible emissions from typical hydrogen flames. It is shown that while visible emissions from these flames are considerably weaker than those from comparable hydrocarbon flames, they are indeed visible, albeit at reduced light levels in most cases. Detailed flame spectra are presented to characterize flame emission bands in the ultraviolet, visible and infrared regions of the spectrum that result in a visible hydrogen flame. The visible blue emission is emphasized, and recorded spectra indicate that fine spectral structure is superimposed on a broadband continuum extending from the ultraviolet into the visible region. Tests were performed to show that this emission does not arise from carbon or nitrogen chemistry resulting from carbon-containing impurities (hydrocarbons) in the hydrogen fuel or from CO{sub 2} or N{sub 2} entrainment from the surrounding air. The spectral structure, however, is also observed in methane flames. The magnitude of the broadband emission increases with flame temperature in a highly nonlinear manner while the finer spectral structure is insensitive to temperature. A comparison of diffusion and premixed H{sub 2} flames shows that the fine scale structure is comparable in both flames. (author)

  20. Numerical Study of Buoyancy and Differential Diffusion Effects on the Structure and Dynamics of Triple Flames

    NASA Technical Reports Server (NTRS)

    Chen, J. -Y.; Echekki, T.

    1999-01-01

    Triple flames arise in a number of practical configurations where fuel and oxidizer are partially premixed, such as in the base of a lifted jet flame. Past experimental studies, theoretical analyses, and numerical modeling of triple flames suggested the potential role of triple flames in stabilizing turbulent flames and in promoting flame propagation. From recent numerical simulations of laminar triple flames, a strong influence of differential diffusion among species and heat on the triple flame structure has been gradually appreciated. This paper reports preliminary numerical results on the influence of gravity and differential diffusion effects on the structure and dynamics of triple flames with a one-step global irreversible chemistry model.

  1. Bunsen flame hydrodynamics

    SciTech Connect

    Wagner, T.C.; Ferguson, C.R.

    1985-01-01

    An investigation into the structure of premixed Bunsen flames was performed to determine whether by using laser velocimetry an unambiguous means of measuring laminar flame speed could be devised and to provide data by which theoreticians could critically evaluate their predictions. Data presented for the former include the axisymmetric flow field and a comparison of cone angles obtained from direct and schlieren photographs of the flame. Data presented for the latter include, for varying equivalence ratios and cone angles, the radius of curvature of the tip and change in velocity through the tip. The centerline velocity was found to decay as a function of axial distance, and a noncoincidence of schlieren and luminous surfaces was observed. When normalized by a preheat thickness (based on the harmonic mean of the thermal conductivity), the behavior of the radius of curvature of the tip compared well with a recent theoretical prediction. 13 references, 5 figures.

  2. Pdf prediction of supersonic hydrogen flames

    NASA Technical Reports Server (NTRS)

    Eifler, P.; Kollmann, W.

    1993-01-01

    A hybrid method for the prediction of supersonic turbulent flows with combustion is developed consisting of a second order closure for the velocity field and a multi-scalar pdf method for the local thermodynamic state. It is shown that for non-premixed flames and chemical equilibrium mixture fraction, the logarithm of the (dimensionless) density, internal energy per unit mass and the divergence of the velocity have several advantages over other sets of scalars. The closure model is applied to a supersonic non-premixed flame burning hydrogen with air supplied by a supersonic coflow and the results are compared with a limited set of experimental data.

  3. Modelling of turbulent lifted jet flames using flamelets: a priori assessment and a posteriori validation

    NASA Astrophysics Data System (ADS)

    Ruan, Shaohong; Swaminathan, Nedunchezhian; Darbyshire, Oliver

    2014-03-01

    This study focuses on the modelling of turbulent lifted jet flames using flamelets and a presumed Probability Density Function (PDF) approach with interest in both flame lift-off height and flame brush structure. First, flamelet models used to capture contributions from premixed and non-premixed modes of the partially premixed combustion in the lifted jet flame are assessed using a Direct Numerical Simulation (DNS) data for a turbulent lifted hydrogen jet flame. The joint PDFs of mixture fraction Z and progress variable c, including their statistical correlation, are obtained using a copula method, which is also validated using the DNS data. The statistically independent PDFs are found to be generally inadequate to represent the joint PDFs from the DNS data. The effects of Z-c correlation and the contribution from the non-premixed combustion mode on the flame lift-off height are studied systematically by including one effect at a time in the simulations used for a posteriori validation. A simple model including the effects of chemical kinetics and scalar dissipation rate is suggested and used for non-premixed combustion contributions. The results clearly show that both Z-c correlation and non-premixed combustion effects are required in the premixed flamelets approach to get good agreement with the measured flame lift-off heights as a function of jet velocity. The flame brush structure reported in earlier experimental studies is also captured reasonably well for various axial positions. It seems that flame stabilisation is influenced by both premixed and non-premixed combustion modes, and their mutual influences.

  4. Premixed Gas Combustion: An Excitable System

    NASA Technical Reports Server (NTRS)

    Pearlman, Howard

    1997-01-01

    Rotating spiral and target patterns have been observed experimentally on freely-propagating premixed gas flames in large diameter tubes at normal gravity (1-g). These modes of propagation occur in near-limit mixtures which have a Lewis number (Le, defined as the ratio of the thermal diffusivity of the cold mixture to the mass diffusivity of the scarce component into the mixture) sufficiently greater than one. However, at 1-g, buoyant flows strongly distort the flame curvature, hydrodynamics (thus stretch) and convective transport of species and heat. In turn, these alter the critical Le required for onset of instability. To isolate and better understand the mechanisms which drive the observed patterns and their dynamics, 1-g and microgravity (micro-g) experiments are being conducted to determine: (1) the structure and dynamics of the patterns, (2) a map of the critical Le and heat loss for their occurrence, (3) the relative significance of the chemical kinetics, and (4) the effect of curvature (local wave and global flame front) on wave propagation. With this in hand, we will be better prepared to discuss an additional mode, a state of 'chemical turbulence,' which seems to be the ultimate fate of many of these near-limit flames prior to extinction.

  5. Oscillating edge-flames

    NASA Astrophysics Data System (ADS)

    Buckmaster, J.; Zhang, Yi

    1999-09-01

    It has been known for some years that when a near-limit flame spreads over a liquid pool of fuel, the edge of the flame can oscillate. It is also known that when a near-asphyxiated candle-flame burns in zero gravity, the edge of the (hemispherical) flame can oscillate violently prior to extinction. We propose that these oscillations are nothing more than a manifestation of the large Lewis number instability well known in chemical reactor studies and in combustion studies, one that is exacerbated by heat losses. As evidence of this we examine an edge-flame confined within a fuel-supply boundary and an oxygen-supply boundary, anchored by a discontinuity in data at the fuel-supply boundary. We show that when the Lewis number of the fuel is 2, and the Lewis number of the oxidizer is 1, oscillations of the edge occur when the Damköhler number is reduced below a critical value. During a single oscillation period there is a short premixed propagation stage and a long diffusion stage, behaviour that has been observed in flame spread experiments. Oscillations do not occur when both Lewis numbers are equal to 1.

  6. Flame Propagation in Low-Intensity Turbulence under Microgravity Conditions

    NASA Technical Reports Server (NTRS)

    Aldredge, R. C.

    2001-01-01

    The goal of the research is to understand the influences of the hydrodynamic instability on premixed-flame propagation. It is known that coupling between flame and flow-field dynamics in association with the hydrodynamic instability may lead to flame-generated turbulence, flame acceleration and enhancement of burning rates. As a result of such hydrodynamic coupling the transition from initially planar or wrinkled laminar flames to fast turbulent flames or detonations is possible, even when diffusive-thermal effects associated with non-unity reactant Lewis numbers are not destabilizing. It is important to identify methods of suppressing the hydrodynamic instability so as to insure fire safety, particularly in space.

  7. Partially premixed prevalorized kerosene spray combustion in turbulent flow

    SciTech Connect

    Chrigui, M.; Ahmadi, W.; Sadiki, A.; Janicka, J.; Moesl, K.

    2010-04-15

    A detailed numerical simulation of kerosene spray combustion was carried out on a partially premixed, prevaporized, three-dimensional configuration. The focus was on the flame temperature profile dependency on the length of the pre-vaporization zone. The results were analyzed and compared to experimental data. A fundamental study was performed to observe the temperature variation and flame flashback. Changes were made to the droplet diameter, kerosene flammability limits, a combustion model parameter and the location of the combustion initialization. Investigations were performed for atmospheric pressure, inlet air temperature of 90 C and a global equivalence ratio of 0.7. The simulations were carried out using the Eulerian Lagrangian procedure under a fully two-way coupling. The Bray-Moss-Libby model was adjusted to account for the partially premixed combustion. (author)

  8. Development of an ion attachment mass spectrometer for direct detection of intermediates in combustion flames.

    PubMed

    Torii, Takahiro; Nishimura, Takashi; Nakamura, Megumi; Shiokawa, Yoshiro; Matsumoto, Kozo; Kitagawa, Kuniyuki

    2008-11-01

    A system with Li+ ion attachment (IA) ionization has been developed for the direct detection of intermediates formed in burning flames by mass spectrometry. Dimethyl ether (DME) among alternative fuels was selected as a test substance to examine the capability of the system. As a result, intermediates generated in a premixed DME-air flame were directly detectable as Li+ adduct ions. By moving the burner on an X-Y stage, spatial distribution profiles of different species, including unburned DME and formaldehyde, were obtained for three types of flames: diffusion, partially premixed, and premixed.

  9. Analysis of Lean Premixed/Prevaporized Combustion with KIVA-2

    NASA Technical Reports Server (NTRS)

    Deur, J. M.; Kundu, K. P.; Darling, D. D.; Cline, M. C.; Micklow, G. J.; Harper, M. R.; Simons, T. A.

    1994-01-01

    Requirements to reduce the emissions of pollutants from gas turbines used in aircraft propulsion and ground based power generation have led to consideration of lean premixed/prevaporized (LPP) combustion concept. This paper describes some of the LPP flame tube analyses performed at the NASA Research Center with KIVA-2, a well-known multi-dimensional CFD code for problems including sprays, turbulence, and combustion. Modifications to KIVA-2's boundary condition and chemistry treatments have been made to meet the needs of the present study. The study itself focuses on two key aspects of the LPP concept, low emissions and flame stability (including flashback and lean blowoff.

  10. Flame tolerant secondary fuel nozzle

    SciTech Connect

    Khan, Abdul Rafey; Ziminsky, Willy Steve; Wu, Chunyang; Zuo, Baifang; Stevenson, Christian Xavier

    2015-02-24

    A combustor for a gas turbine engine includes a plurality of primary nozzles configured to diffuse or premix fuel into an air flow through the combustor; and a secondary nozzle configured to premix fuel with the air flow. Each premixing nozzle includes a center body, at least one vane, a burner tube provided around the center body, at least two cooling passages, a fuel cooling passage to cool surfaces of the center body and the at least one vane, and an air cooling passage to cool a wall of the burner tube. The cooling passages prevent the walls of the center body, the vane(s), and the burner tube from overheating during flame holding events.

  11. Development of Criteria for Flameholding Tendencies within Premixer Passages for High Hydrogen Content Fuels

    SciTech Connect

    Lewis, Elliot; McDonell, Vincent

    2015-03-31

    Due to increasingly stringent air quality requirements stationary power gas turbines have moved to lean-premixed operation, which reduces pollutant emissions but can result in flashback. Flashback can cause serious damage to the premixer hardware. Curtailing flashback can be difficult with hydrocarbon fuels and becomes even more challenging when hydrogen is used as the fuel. The two main approaches for coping with flashback are either to design a combustor that is resistant to flashback, or to design a premixer that will not anchor a flame if flashback occurs. Even with a well-designed combustor flashback can occur under certain circumstances, thus it is necessary to determine how to avoid flameholding within the premixer passageways of a gas turbine. To this end, an experiment was designed that would determine the flameholding propensities at elevated pressures and temperatures of three different classes of geometric features commonly found in gas turbine premixers, with both natural gas and hydrogen fuel. Experiments to find the equivalence ratio at blow off were conducted within an optically accessible test apparatus with four flameholders: 0.25 and 0.50 inch diameter cylinders, a reverse facing step with a height of 0.25 inches, and a symmetric airfoil with a thickness of 0.25 inches and a chord length of one inch. Tests were carried out at temperatures between 300 K and 750 K, at pressures up to 9 atmospheres. Typical bulk velocities were between 40 and 100 m/s. The effect of airfoil’s angle of rotation was also investigated. Blow off for hydrogen flames was found to occur at much lower adiabatic flame temperatures than natural gas flames. Additionally it was observed that at high pressures and high turbulence intensities, reactant velocity does not have a noticeable effect on the point of blow off due in large part to corresponding increases in turbulent flame speed. Finally a semi empirical correlation was developed that predicts flame extinction for both

  12. Gravitational Effects on Cellular Flame Structure

    NASA Technical Reports Server (NTRS)

    Dunsky, C. M.; Fernandez-Pello, A. C.

    1991-01-01

    An experimental investigation has been conducted of the effect of gravity on the structure of downwardly propagating, cellular premixed propane-oxygen-nitrogen flames anchored on a water-cooled porous-plug burner. The flame is subjected to microgravity conditions in the NASA Lewis 2.2-second drop tower, and flame characteristics are recorded on high-speed film. These are compared to flames at normal gravity conditions with the same equivalence ratio, dilution index, mixture flow rate, and ambient pressure. The results show that the cellular instability band, which is located in the rich mixture region, changes little under the absence of gravity. Lifted normal-gravity flames near the cellular/lifted limits, however, are observed to become cellular when gravity is reduced. Observations of a transient cell growth period following ignition point to heat loss as being an important mechanism in the overall flame stability, dominating the stabilizing effect of buoyancy for these downwardly-propagating burner-anchored flames. The pulsations that are observed in the plume and diffusion flame generated downstream of the premixed flame in the fuel rich cases disappear in microgravity, verifying that these fluctuations are gravity related.

  13. Lean Premixed Combustion Stabilized by Low Swirl a Promising Concept for Practical Applications

    NASA Technical Reports Server (NTRS)

    Cheng, R. K.

    1999-01-01

    Since its inception, the low-swirl burner (LSB) has shown to be a useful laboratory apparatus for fundamental studies of premixed turbulent flames. The LSB operates under wide ranges of equivalence ratios, flow rates, and turbulence intensities. Its flame is lifted and detached from the burner and allows easy access for laser diagnostics. The flame brush is axisymmetric and propagates normal to the incident reactants. Therefore, the LSB is well suited for investigating detailed flame structures and empirical coefficients such as flame speed, turbulence transport, and flame generated turbulence. Due to its capability to stabilize ultra-lean premixed turbulent flames (phi approx. = 0.55), the LSB has generated interest from the gas appliance industry for use as an economical low-NO(x) burner. Lean premixed combustion emits low levels of NO(x), due primarily to the low flame temperature. Therefore, it is a very effective NO(x) prevention method without involving selective catalytic reduction (SCR), fuel-air staging, or flue gas recirculation (FGR). En the gas turbine industry, substantial research efforts have already been undertaken and engines with lean premixed combustors are already in use. For commercial and residential applications, premixed pulsed combustors and premixed ceramic matrix burners are commercially available. These lean premixed combustion technologies, however, tend to be elaborate but have relatively limited operational flexibility, and higher capital, operating and maintenance costs. Consequently, these industries are continuing the development of lean premixed combustion technologies as well as exploring new concepts. This paper summarizes the research effects we have undertaken in the past few years to demonstrate the feasibility of applying the low-swirl flame stabilization method for a wide range of heating and power generation systems. The principle of flame stabilization by low-swirl is counter to the conventional high-swirl methods that

  14. Turbulent Nonpremixed Flames (TNF): Experimental Data Archives and Computational Submodels

    DOE Data Explorer

    In the 1990s an international collaboration formed around a series of workshops that became known collectively as the International Workshop on Measurement and Computation of Turbulent Non-Premixed Flames (TNF). An online library, hosted by Sandia National Laboratory (California) was established that provides data sets and submodels or "mechanisms" for the study of turbulence-chemistry interactions in turbulent nonpremixed and partially premixed combustion. Data are organized by flame types: simple jet flames, piloted jet flames, bluff body flames, and swirl flames. These data sets provide a means for collaborative comparisons of both measured and simulated/modeled research results and also assist scientists in determining priorities for further research. More than 20 data sets or databases are available from this website, along with various downloadable files of chemical mechanisms. The website also provides an extensive bibliography and the proceedings of the workshops themselves from 1996 through 2012. Information continues to be added to this collection.

  15. Stratified turbulent Bunsen flames: flame surface analysis and flame surface density modelling

    NASA Astrophysics Data System (ADS)

    Ramaekers, W. J. S.; van Oijen, J. A.; de Goey, L. P. H.

    2012-12-01

    In this paper it is investigated whether the Flame Surface Density (FSD) model, developed for turbulent premixed combustion, is also applicable to stratified flames. Direct Numerical Simulations (DNS) of turbulent stratified Bunsen flames have been carried out, using the Flamelet Generated Manifold (FGM) reduction method for reaction kinetics. Before examining the suitability of the FSD model, flame surfaces are characterized in terms of thickness, curvature and stratification. All flames are in the Thin Reaction Zones regime, and the maximum equivalence ratio range covers 0.1⩽φ⩽1.3. For all flames, local flame thicknesses correspond very well to those observed in stretchless, steady premixed flamelets. Extracted curvature radii and mixing length scales are significantly larger than the flame thickness, implying that the stratified flames all burn in a premixed mode. The remaining challenge is accounting for the large variation in (subfilter) mass burning rate. In this contribution, the FSD model is proven to be applicable for Large Eddy Simulations (LES) of stratified flames for the equivalence ratio range 0.1⩽φ⩽1.3. Subfilter mass burning rate variations are taken into account by a subfilter Probability Density Function (PDF) for the mixture fraction, on which the mass burning rate directly depends. A priori analysis point out that for small stratifications (0.4⩽φ⩽1.0), the replacement of the subfilter PDF (obtained from DNS data) by the corresponding Dirac function is appropriate. Integration of the Dirac function with the mass burning rate m=m(φ), can then adequately model the filtered mass burning rate obtained from filtered DNS data. For a larger stratification (0.1⩽φ⩽1.3), and filter widths up to ten flame thicknesses, a β-function for the subfilter PDF yields substantially better predictions than a Dirac function. Finally, inclusion of a simple algebraic model for the FSD resulted only in small additional deviations from DNS data

  16. Development of lean premixed low-swirl burner for low NO{sub x} practical application

    SciTech Connect

    Yegian, D.T.; Cheng, R.K.

    1999-07-07

    Laboratory experiments have been performed to evaluate the performance of a premixed low-swirl burner (LSB) in configurations that simulate commercial heating appliances. Laser diagnostics were used to investigate changes in flame stabilization mechanism, flowfield, and flame stability when the LSB flame was confined within quartz cylinders of various diameters and end constrictions. The LSB adapted well to enclosures without generating flame oscillations and the stabilization mechanism remained unchanged. The feasibility of using the LSB as a low NO{sub x} commercial burner has also been verified in a laboratory test station that simulates the operation of a water heater. It was determined that the LSB can generate NO{sub x} emissions < 10 ppm (at 3% O{sub 2}) without significant effect on the thermal efficiency of the conventional system. The study has demonstrated that the lean premixed LSB has commercial potential for use as a simple economical and versatile burner for many low emission gas appliances.

  17. Structure Of Flame Balls At Low Lewis-number (SOFBALL)

    NASA Technical Reports Server (NTRS)

    Ronney, Paul D.

    1995-01-01

    The work has encompassed several topics related to the experimental and theoretical study of combustion limits in premixed flames at microgravity. These topics include (1) flame structure and stability at low Lewis number (which is the basis for the SOFBALL space flight experiment), (2) flame propagation and extinction in cylindrical tubes, and (3) experimental simulation of combustion processes using autocatalytic chemical reactions. Progress on each of these topics is outlined.

  18. Successive laser ablation ignition of premixed methane/air mixtures.

    PubMed

    Bak, Moon Soo; Cappelli, Mark A

    2015-06-01

    Laser ablation has been used to study successive ignition in premixed methane/air mixtures under conditions in which the flow speed leads to flame blow-out. A range of laser pulse frequencies is experimentally mimicked by varying the time interval between two closely spaced laser pulses. Emission intensities from the laser ablation kernels are measured to qualitatively estimate laser energy coupling, and flame CH* chemiluminescence is recorded in a time-resolved manner to capture the flame evolution and propagation. A comparison of the measurements is made between the two successive breakdown ignition events. It is found that the formation of the subsequent ablation kernel is almost independent of the previous one, however, for the successive breakdowns, the first breakdown and its ensuing combustion created temporal regions of no energy coupling as they heat the gas and lower the density. Flame imaging shows that the second ablation event successfully produces another flame kernel and is capable of holding the flame-base even at pulse intervals where the second laser pulse cannot form a breakdown. This study demonstrates that successive ablation ignition can allow for the use of higher laser frequencies and enhanced flame stabilization than successive breakdown ignition. PMID:26072866

  19. Cinema particle image velocimetry investigation of turbulent jet flame stabilization

    NASA Astrophysics Data System (ADS)

    Upatnieks, Ansis

    A new cinema PIV system was developed and used to study the physical phenomena of non-premixed turbulent jet flame stabilization. The system offers an unprecedented combination of image acquisition rate (8000/s), sequence length (4000) and resolution (equivalent to 1K x 1.5K pixels) that provides finely resolved yet extraordinarily lengthy time histories of the evolution of velocity fields in laboratory-scale gas-phase turbulent flows. These measurements provide quantitative information concerning the dynamics of turbulence and combustion that is not available from conventional experimental techniques or computational simulations. For example, time histories of the interaction between turbulent vortex structures and the flame thermal boundary are observed. Gas and flame velocities are obtained simultaneously, yielding direct measurements of flame propagation velocities. The gas and flame velocities are highly correlated, suggesting strong interaction between the velocity field and the flame. The gas and propagation velocities at the flame base remain close to premixed laminar burning velocities (SL), which are three to four times smaller than the velocities in corresponding non-reacting cases. Strong reverse flow is observed upstream of the flame base, suggesting that the velocity reduction is caused by heat release-induced dilatation. These observations suggest that the dilatation velocity field plays a dominant role in stabilization by reducing incident gas velocities to levels at which laminar premixed, triple, or edge flames can be sustained.

  20. Large eddy simulation of a lifted turbulent jet flame

    SciTech Connect

    Ferraris, S.A.; Wen, J.X.

    2007-09-15

    The flame index concept for large eddy simulation developed by Domingo et al. [P. Domingo, L. Vervisch, K. Bray, Combust. Theory Modell. 6 (2002) 529-551] is used to capture the partially premixed structure at the leading point and the dual combustion regimes further downstream on a turbulent lifted flame, which is composed of premixed and nonpremixed flame elements each separately described under a flamelet assumption. Predictions for the lifted methane/air jet flame experimentally tested by Mansour [M.S. Mansour, Combust. Flame 133 (2003) 263-274] are made. The simulation covers a wide domain from the jet exit to the far flow field. Good agreement with the data for the lift-off height and the mean mixture fraction has been achieved. The model has also captured the double flames, showing a configuration similar to that of the experiment which involves a rich premixed branch at the jet center and a diffusion branch in the outer region which meet at the so-called triple point at the flame base. This basic structure is contorted by eddies coming from the jet exit but remains stable at the lift-off height. No lean premixed branches are observed in the simulation or and experiment. Further analysis on the stabilization mechanism was conducted. A distinction between the leading point (the most upstream point of the flame) and the stabilization point was made. The later was identified as the position with the maximum premixed heat release. This is in line with the stabilization mechanism proposed by Upatnieks et al. [A. Upatnieks, J. Driscoll, C. Rasmussen, S. Ceccio, Combust. Flame 138 (2004) 259-272]. (author)

  1. LES and acoustic analysis of thermo-acoustic instabilities in a partially premixed model combustor

    NASA Astrophysics Data System (ADS)

    Hernández, Ignacio; Staffelbach, Gabriel; Poinsot, Thierry; Román Casado, Juan C.; Kok, Jim B. W.

    2013-01-01

    Numerical simulations were performed using Large Eddy Simulation (LES) and acoustic analysis tools to study thermo-acoustic instabilities in a methane/air academic burner installed at the University of Twente (The Netherlands). It operates under fuel-lean partially premixed conditions at atmospheric pressure, and was built to study thermo-acoustic instabilities in conditions representative of gas turbine Lean Premixed systems: gaseous fuel is injected upstream of the combustor and has a limited time to mix with air. Even though the objective is to burn in a premixed mode, the actual regime corresponds to a partially premixed flame where strong equivalence ratio variations are created especially during combustion instabilities. Capturing these modes with LES is a challenge: here, simulations for both stable and unstable regimes are performed. In the unstable case, the limit cycle oscillations (LCO) are characterized and compared to experimental results. Reasonable agreement is found between simulations and experiments.

  2. Mechanisms and enhancement of flame stabilization. Annual report, January 15, 1992--January 14, 1993

    SciTech Connect

    Law, C.K.

    1993-02-01

    During the reporting period, useful contributions have been made in understanding the structure of laminar premixed and diffusion flames, with emphasis on the influence of aerodynamics and chemical kinetics. These contributions include (1) derivation of the missing closure condition for the activation energy asymptotic analysis of premixed flames, (2) identification of a dual extinction mode for radiation-affected flames, (3) formulation of a unified theory of fundamental flammability limits, and (4) demonstration that flame stabilization can be achieved in the absence of heat loss. These investigations have been conducted via experimental, analytical and computational approaches, with strong coupling between the individual components.

  3. Study on the potential of BML-approach and G-equation concept-based models for predicting swirling partially premixed combustion systems: URANS computations

    SciTech Connect

    Schneider, E.; Maltsev, A.; Sadiki, A.; Janicka, J.

    2008-03-15

    In this work the potential of two combustion modeling approaches (BML and G-equation based models) for partially premixed flames in combustion systems of various complexities is investigated using URANS computations. The first configuration consists of a nonconfined swirled premixed methane/air flame (swirl number 0.75) exhibiting partially premixed effects due to coflowing. The system is studied either in the isothermal case or in the reacting mode and for different thermal powers. The second configuration represents a model GT combustion chamber and features the main properties of real GT combustors: a confined swirled flow with multiple recirculation zones and reattachment points, resulting in a partially premixed methane/air aerodynamically stabilized flame and an additional diffusion flame formed by the fuel and oxidizer not consumed in the premixed flame. This makes it possible to subject the modeling to variation of different parameters, such as confinement, Re-number or flame power, or adiabatic or nonadiabatic conditions. For this purpose an extended Bray-Moss-Libby model and a G-equation-based approach, both coupled to the mixture fraction transport equation to account for partially premixed effects, are used following the so-called conditional progress variable approach (CPVA). The radiation effects are also taken into account. To account for the turbulence-chemistry interaction, a (multivariate) presumed PDF approach is applied. The results are compared with LDV, Raman, and PLIF measurements. Beyond a pure validation, the URANS is used to capture the presence of the precessing vortex core and to analyze the performance of different modeling strategies of partially premixed combustion in capturing the expansion ratio, species formation conditioned on the flame front, and flame front stabilization. It appears that the combustion models used are able to achieve plausible results in the complex combustion systems under study, while the BML-based model

  4. Aromatics oxidation and soot formation in flames

    SciTech Connect

    Howard, J.B.; Pope, C.J.; Shandross, R.A.; Yadav, T.

    1993-12-01

    This project is concerned with the kinetics and mechanisms of aromatics oxidation and soot and fullerenes formation in flames. The scope includes detailed measurements of profiles of stable and radical species concentrations in low-pressure one-dimensional premixed flames. Intermediate species identifications and mole fractions, fluxes, and net reaction rates calculated from the measured profiles are used to test postulated reaction mechanisms. Particular objectives are to identify and to determine or confirm rate constants for the main benzene oxidation reactions in flames, and to characterize fullerenes and their formation mechanisms and kinetics.

  5. Turbulent Flame Processes Via Diffusion Flame-Vortex Ring Interactions

    NASA Technical Reports Server (NTRS)

    Dahm, Werner J. A.; Chen, Shin-Juh; Silver, Joel A.; Piltch, Nancy D.; VanderWal, Randall L.

    2001-01-01

    Flame-vortex interactions are canonical configurations that can be used to study the underlying processes occurring in turbulent reacting flows. This configuration contains many of the fundamental aspects of the coupling between fluid dynamics and combustion that could be investigated with more controllable conditions than are possible under direct investigations of turbulent flames. Diffusion flame-vortex ring interaction contains many of the fundamental elements of flow, transport, combustion, and soot processes found in turbulent diffusion flames. Some of these elements include concentrated vorticity, entrainment and mixing, strain and nonequilibrium phenomena, diffusion and differential diffusion, partial premixing and diluent effects, soot formation and oxidation, and heat release effects. Such simplified flowfield allows the complex processes to be examined more closely and yet preserving the physical processes present in turbulent reacting flows. Furthermore, experimental results from the study of flame-vortex interactions are useful for the validation of numerical simulations and more importantly to deepen our understanding of the fundamental processes present in reacting flows. Experimental and numerical results obtained under microgravity conditions of the diffusion flame-vortex ring interaction are summarized in this paper. Results are obtained using techniques that include Flame Luminosity Imaging (FLI), Laser Soot-Mie Scattering (LSMS), Computational Fluid Dynamics and Combustion (CFDC), and Diode Laser Spectroscopy/Iterative Temperature with Assumed Chemistry (DLS/ITAC).

  6. Premixer Design for High Hydrogen Fuels

    SciTech Connect

    Benjamin P. Lacy; Keith R. McManus; Balachandar Varatharajan; Biswadip Shome

    2005-12-16

    This 21-month project translated DLN technology to the unique properties of high hydrogen content IGCC fuels, and yielded designs in preparation for a future testing and validation phase. Fundamental flame characterization, mixing, and flame property measurement experiments were conducted to tailor computational design tools and criteria to create a framework for predicting nozzle operability (e.g., flame stabilization, emissions, resistance to flashback/flame-holding and auto-ignition). This framework was then used to establish, rank, and evaluate potential solutions to the operability challenges of IGCC combustion. The leading contenders were studied and developed with the most promising concepts evaluated via computational fluid dynamics (CFD) modeling and using the design rules generated by the fundamental experiments, as well as using GE's combustion design tools and practices. Finally, the project scoped the necessary steps required to carry the design through mechanical and durability review, testing, and validation, towards full demonstration of this revolutionary technology. This project was carried out in three linked tasks with the following results. (1) Develop conceptual designs of premixer and down-select the promising options. This task defined the ''gap'' between existing design capabilities and the targeted range of IGCC fuel compositions and evaluated the current capability of DLN pre-mixer designs when operated at similar conditions. Two concepts (1) swirl based and (2) multiple point lean direct injection based premixers were selected via a QFD from 13 potential design concepts. (2) Carry out CFD on chosen options (1 or 2) to evaluate operability risks. This task developed the leading options down-selected in Task 1. Both a GE15 swozzle based premixer and a lean direct injection concept were examined by performing a detailed CFD study wherein the aerodynamics of the design, together with the chemical kinetics of the combustion process, were

  7. Effect of fuel mixture fraction and velocity perturbations on the flame transfer function of swirl stabilized flames

    NASA Astrophysics Data System (ADS)

    Wysocki, Stefan; Di-Chiaro, Giacomo; Biagioli, Fernando

    2015-11-01

    A novel methodology is developed to decompose the classic Flame Transfer Function (FTF) used in the thermo-acoustic stability analysis of lean premix combustors into contributions of different types. The approach is applied, in the context of Large Eddy Simulation (LES), to partially-premixed and fully-premixed flames, which are stabilized via a central recirculation zone as a result of the vortex breakdown phenomenon. The first type of decomposition is into contributions driven by fuel mixture fraction and dynamic velocity fluctuations. Each of these two contributions is further split into the components of turbulent flame speed and flame surface area. The flame surface area component, driven by the pure dynamic velocity fluctuation, which is shown to be a dominant contribution to the overall FTF, is also additionally decomposed over the coherent flow structures using proper orthogonal decomposition. Using a simplified model for the dynamic response of premixed flames, it is shown that the distribution of the FTF, as obtained from LES, is closely related to the characteristics of the velocity field frequency response to the inlet perturbation. Initially, the proposed method is tested and validated with a well characterized laboratory burner geometry. Subsequently, the method is applied to an industrial gas turbine burner.

  8. Flame acceleration in the early stages of burning in tubes

    SciTech Connect

    Bychkov, Vitaly; Fru, Gordon; Petchenko, Arkady; Akkerman, V'yacheslav; Eriksson, Lars-Erik

    2007-09-15

    Acceleration of premixed laminar flames in the early stages of burning in long tubes is considered. The acceleration mechanism was suggested earlier by Clanet and Searby [Combust. Flame 105 (1996) 225]. Acceleration happens due to the initial ignition geometry at the tube axis when a flame develops to a finger-shaped front, with surface area growing exponentially in time. Flame surface area grows quite fast but only for a short time. The analytical theory of flame acceleration is developed, which determines the growth rate, the total acceleration time, and the maximal increase of the flame surface area. Direct numerical simulations of the process are performed for the complete set of combustion equations. The simulations results and the theory are in good agreement with the previous experiments. The numerical simulations also demonstrate flame deceleration, which follows acceleration, and the so-called ''tulip flames''. (author)

  9. A dynamic model for the turbulent burning velocity for large eddy simulation of premixed combustion

    SciTech Connect

    Knudsen, E.; Pitsch, H.

    2008-09-15

    Turbulent premixed combustion is particularly difficult to describe using large eddy simulation (LES). In LES, premixed flame structures typically exist on subfilter length scales. Consequently, premixed LES models must be capable of describing how completely unresolved flame structures propagate under the influence of completely unresolved eddies. This description is usually accomplished through the implementation of a model for the turbulent burning velocity. Here, a dynamic model for describing the turbulent burning velocity in the context of LES is presented. This model uses a new surface filtering procedure that is consistent with standard LES filtering. Additionally, it only uses information that comes directly from the flame front. This latter attribute is important for two reasons. First, it guarantees that the model can be consistently applied when level set methods, where arbitrary constraints can be imposed on field variables away from fronts, are used to track the flame. Second, it forces the model to recognize that the physics governing flame front propagation are only valid locally at the front. Results showing model validation in the context of direct numerical simulation (DNS), and model application in the context of LES, are presented. (author)

  10. Effects Of Ignition on Premixed Vortex Rings: A Simultaneous PLIF and PIV Investigation

    NASA Astrophysics Data System (ADS)

    Meyer, T. R.; Gord, J. R.; Katta, V. R.; Gogineni, S. P.

    2001-11-01

    Preliminary studies of reacting, premixed vortex rings have shown that flame propagation is highly sensitive to ignition timing, equivalence ratio, and vortex strength. A variety of divergent phenomena have been observed, such as interior/exterior flame propagation, vortex-induced flame bridging across the jet column, and the formation of unburned pockets. In the current work, planar laser-induced fluorescence (PLIF) of acetone and OH is performed to study the non-reacting and reacting regions, respectively, and particle image velocimetry (PIV) is used to study the effects of reaction on the flow field. The flow field consists of well-characterized vortex rings of premixed methane and air generated at the exit of an axisymmetric nozzle using a solenoid-driven piston. Ignition is initiated at various phases of vortex development and propagation. Results are compared with corresponding numerical simulations from a time-dependent computational fluid dynamics code with chemistry.

  11. Premixed turbulent combustion to opposed streams

    SciTech Connect

    Kostiuk, L.W.; Cheng, R.K.

    1992-03-01

    Premixed turbulent combustion in opposed streams has been studied experimentally by the use of two component laser doppler aneomometry. This flow geometry is part of a class of stagnating flows used to study turbulent combustion in recent years. It does not involve any surface near the flames because of the flow symmetry thus circumventing many of the effects of flame surface interaction. The mean non-reacting flow is found to be self-similar for all the conditions studied in this and the stagnation plate configuration. A homogeneous region of plane straining is produced in the vicinity of the stagnation and there is a strong interaction between the turbulence in the flow and the mean straining which can increase the rms velocity as the flow stagnates. The reacting flow fields are found to be symmetric about the free stagnation point. The traverses of mean axial velocity in the stagnation streamlines for reaction flows are not dramatically different from the non-reaction flows. These results differ from turbulent combustion experiments where the flow is stagnated by a flat plate. The extinction limits was studied for propane:air mixtures. 11 refs.

  12. Flame-vortex interactions imaged in microgravity

    NASA Technical Reports Server (NTRS)

    Driscoll, James F.; Dahm, Werner J. A.; Sichel, Martin

    1995-01-01

    The scientific objective is to obtain high quality color-enhanced digital images of a vortex exerting aerodynamic strain on premixed and nonpremixed flames with the complicating effects of buoyancy removed. The images will provide universal (buoyancy free) scaling relations that are required to improve several types of models of turbulent combustion, including KIVA-3, discrete vortex, and large-eddy simulations. The images will be used to help quantify several source terms in the models, including those due to flame stretch, flame-generated vorticity, flame curvature, and preferential diffusion, for a range of vortex sizes and flame conditions. The experiment is an ideal way to study turbulence-chemistry interactions and isolate the effect of vortices of different sizes and strengths in a repeatable manner. A parallel computational effort is being conducted which considers full chemistry and preferential diffusion.

  13. Influence of drop size distribution and fuel vapor fraction on premixed spray combustion

    NASA Astrophysics Data System (ADS)

    Machiroutu, Sridhar Venkatabojji

    Premixed spray combustion is affected by fuel and oxidizer properties, mixture equivalence ratio and spray quality. The spray quality is characterized by a mean droplet diameter (SMD) and a droplet size distribution (DSD). Prior experimental studies have considered only the influence of SMD, in part due to the difficulty in controlling the DSD independently. The present work provides experimental evidence demonstrating the effect of the fuel droplet size distribution and fuel vapor fraction on premixed spray combustion. Combustion experiments were performed in a pilot-ignited, continuous flow, tubular, vertical test rig wherein fuel sprays were injected into an air stream. A novel twin-atomizer technique that allowed control over overall equivalence ratio, SMD, DSD, and fuel vapor fraction of the premixed spray was used to generate test sprays. A line-of-sight, infrared (IR) extinction technique was developed to quantify the fuel vapor fraction in premixed sprays. Radial distributions of fuel vapor were evaluated using an 'onion peeling' deconvolution technique. Combustion of test sprays indicated flame propagation among regions of high fuel vapor fraction to generate a high rate of combustion. In lean premixed sprays, the presence of a low fuel vapor concentration does not impact the combustion process. Experimental evidence demonstrating the enhancement of flame propagation velocity for optimal SMDs of ethanol sprays has been found. It was observed that test sprays with narrower DSDs have faster burning rates and more complete combustion. The DSD of the sprays were characterized with a droplet surface-area-based standard deviation of the DSD.

  14. Stretch-rate relationships for turbulent premixed combustion LES subgrid models measured using temporally resolved diagnostics

    SciTech Connect

    Steinberg, Adam M.; Driscoll, James F.

    2010-07-15

    Temporally resolved measurements of turbulence-flame interaction were used to experimentally determine relationships for the strain-rate and curvature stretch-rate exerted on a premixed flame surface. These relationships include a series of transfer functions that are analogous to, but not equal to, stretch-efficiency functions. The measurements were obtained by applying high-repetition-rate particle image velocimetry in a turbulent slot Bunsen flame and were able to resolve the range of turbulent scales that cause flame surface straining and wrinkling. Fluid control masses were tracked in a Lagrangian manner as they interacted with the flame surface. From each interaction, the spatially and temporally filtered subgrid strain-rate and curvature stretch-rate were measured. By analyzing the statistics of thousands of turbulence-flame interactions, relationships for the strain-rate and curvature stretch-rate were determined that are appropriate for Large Eddy Simulation. It was found that the strain-rate exerted on the flame during these interactions was better correlated with the strength of the subgrid fluid-dynamic strain-rate field than with previously used characteristic strain-rates. Furthermore, stretch-efficiency functions developed from simplified vortex-flame interactions significantly over-predict the measurements. Hence, the proposed relationship relates the strain-rate on the flame to the filtered subgrid fluid-dynamic strain-rate field during real turbulence-flame interactions using an empirically determined Strain-Rate Transfer function. It was found that the curvature stretch-rate did not locally balance the strain-rate as has been proposed in previous models. A geometric relationship was found to exist between the subgrid flame surface wrinkling factor and subgrid curvature stretch-rate, which could be expressed using an empirically determined wrinkling factor transfer function. Curve fits to the measured relationships are provided that could be

  15. Lean premixed/prevaporized combustion

    NASA Technical Reports Server (NTRS)

    Lefebvre, A. H. (Editor)

    1977-01-01

    Recommendations were formulated on the status and application of lean premixed/prevaporized combustion to the aircraft gas turbine for the reduction of pollutant emissions. The approach taken by the NASA Stratospheric Cruise Emission Reduction Program (SCERP) in pursuing the lean premixed/prevaporized combustion technique was also discussed. The proceedings contains an overview of the SCERP program, the discussions and recommendations of the participants, and an overall summary.

  16. Flame Chemiluminescence Rate Constants for Quantitative Microgravity Combustion Diagnostics

    NASA Technical Reports Server (NTRS)

    Luque, Jorge; Smith, Gregory P.; Jeffries, Jay B.; Crosley, David R.; Weiland, Karen (Technical Monitor)

    2001-01-01

    Absolute excited state concentrations of OH(A), CH(A), and C2(d) were determined in three low pressure premixed methane-air flames. Two dimensional images of chemiluminescence from these states were recorded by a filtered CCD camera, processed by Abel inversion, and calibrated against Rayleigh scattering, Using a previously validated 1-D flame model with known chemistry and excited state quenching rate constants, rate constants are extracted for the reactions CH + O2 (goes to) OH(A) + CO and C2H + O (goes to) CH(A) + CO at flame temperatures. Variations of flame emission intensities with stoichiometry agree well with model predictions.

  17. An experimental investigation of flame behavior during cylindrical vessel explosions

    SciTech Connect

    Starke, R.; Roth, P.

    1986-12-01

    The propagation of premixed flames centrally ignited at one of the end flanges of a closed cylindrical vessel and the flame-induced fluid flow have been investigated in the present study. Photographic records show that under specific geometrical conditions the flame exhibits a cone form with a backward directed top, called ''tulip'' -shaped. This appears after the flame has lost a main part of its area by side wall quenching. With a laser-Doppler anemometer the instantaneous flow velocity during the short explosion process was measured together with pressure records.

  18. An experimental investigation of flame behavior during cylindrical vessel explosions

    NASA Astrophysics Data System (ADS)

    Starke, R.; Roth, P.

    1986-12-01

    The propagation of premixed flames centrally ignited at one of the end flanges of a closed cylindrical vessel and the flame-induced flow have been investigated. Photographic records show that under specific geometrical conditions the flame exhibits a cone form with a backward directed top, called tulip-shaped. This appears after the flame has lost a main part of its area by side wall quenching. The instantaneous flow velocity during the short explosion process was measured, together with pressure records, with an LDV. An analogy to the experiments of Markstein (1964), is shown, and the explanations of several authors for the 'tulip' formation are given.

  19. Experimental study of turbulent flame kernel propagation

    SciTech Connect

    Mansour, Mohy; Peters, Norbert; Schrader, Lars-Uve

    2008-07-15

    Flame kernels in spark ignited combustion systems dominate the flame propagation and combustion stability and performance. They are likely controlled by the spark energy, flow field and mixing field. The aim of the present work is to experimentally investigate the structure and propagation of the flame kernel in turbulent premixed methane flow using advanced laser-based techniques. The spark is generated using pulsed Nd:YAG laser with 20 mJ pulse energy in order to avoid the effect of the electrodes on the flame kernel structure and the variation of spark energy from shot-to-shot. Four flames have been investigated at equivalence ratios, {phi}{sub j}, of 0.8 and 1.0 and jet velocities, U{sub j}, of 6 and 12 m/s. A combined two-dimensional Rayleigh and LIPF-OH technique has been applied. The flame kernel structure has been collected at several time intervals from the laser ignition between 10 {mu}s and 2 ms. The data show that the flame kernel structure starts with spherical shape and changes gradually to peanut-like, then to mushroom-like and finally disturbed by the turbulence. The mushroom-like structure lasts longer in the stoichiometric and slower jet velocity. The growth rate of the average flame kernel radius is divided into two linear relations; the first one during the first 100 {mu}s is almost three times faster than that at the later stage between 100 and 2000 {mu}s. The flame propagation is slightly faster in leaner flames. The trends of the flame propagation, flame radius, flame cross-sectional area and mean flame temperature are related to the jet velocity and equivalence ratio. The relations obtained in the present work allow the prediction of any of these parameters at different conditions. (author)

  20. An elementary discussion of propellant flame geometry

    SciTech Connect

    Buckmaster, J.; Jackson, T.L.; Yao, J.

    1999-05-01

    The authors examine the geometry of diffusion flames generated by the burning of a heterogeneous solid propellant, using a simple model designed to provide qualitative insights. In the fast chemistry limit a strategy is used which has its roots in Burke and Schumann`s 1928 study of diffusion flames, albeit with different boundary conditions. This shows that the stoichiometric level surface (SLS) intersects the propellant surface at a point displaced from the fuel/oxidizer interface, and the variations of this displacement with Peclet number are discussed. The authors show that for model sandwich propellants, or their axisymmetric counterpart, the geometry of the SLS when the core is oxidizer is quite different from the geometry of the SLS when the core is fuel. Also, it is much easier to quench the flame on an oxidizer core, by reducing the Peclet number, than it is to quench the flame on a fuel core. When finite chemistry effects are accounted for, the flame only occupies a portion of the SLS, and there is a leading edge structure in which premixing plays a role. Enhancement of the burning rate due to premixing is identified, but a well-defined tribrachial structure is not observed. The authors show how a sharp reduction in pressure can lead to a detachment of the flame from the SLS, with subsequent quenching as it is swept downstream.

  1. Flame Inhibition by Phosphorus-Containing Compounds in Lean and Rich Propane Flames

    SciTech Connect

    Curran, H; Korobeinichev, O P; Shvartsberg, V M; Shmakov, A G; Bolshova, T A; Jayaweera, T M; Melius, C F; Pitz, W J; Westbrook, C K

    2003-12-19

    Chemical inhibition of laminar propane flames by organophosphorus compounds has been studied experimentally, using a laboratory Mache Hebra nozzle burner and a flat flame burner with molecular beam mass spectrometry (MBMS), and with a computational flame model using a detailed chemical kinetic reaction mechanism. Both fuel-lean and fuel-rich propane flames were studied to examine the role of equivalence ratio in flame inhibition. The experiments examined a wide variety of organophosphorus compounds. We report on the experimental species flame profiles for tri-methyl phosphate (TMP) and compare them with the species flame profile results from modeling of TMP and di-methyl methyl phosphonate (DMMP). Both the experiments and kinetic modeling support and illustrate previous experimental studies in both premixed and non-premixed flames that inhibition efficiency is effectively the same for all of the organophosphorus compounds examined, independent of the molecular structure of the initial inhibitor molecule. The chemical inhibition is due to reactions involving the small P-bearing species HOPO{sub 2} and HOPO that are produced by the organophosphorus compounds (OPCs). The ratios of the HOPO{sub 2} and HOPO concentrations differ between the lean and rich flames, with HOPO{sub 2} dominant in lean flames while HOPO dominates in rich flames. The resulting HOPO{sub 2} and HOPO species profiles do not depend significantly on the initial source of the HOPO{sub 2} and HOPO and thus are relatively insensitive to the initial OPC inhibitor. A more generalized form of the original Twarowski mechanism for hydrocarbon radical recombination is developed to account for the results observed, and new theoretical values have been determined for heats of formation of the important P-containing species, using the BAC-G2 method.

  2. Effects of fuel type and equivalence ratios on the flickering of triple flames

    SciTech Connect

    Sahu, K.B.; Kundu, A.; Ganguly, R.; Datta, A.

    2009-02-15

    An experimental study has been conducted in axisymmetric, co-flowing triple flames with different equivalence ratios of the inner and outer reactant streams (2<{phi}{sub in}<3 and 0{<=}{phi}{sub out}<0.7). Different fuel combinations, like propane/propane, propane/methane or methane/methane in the inner and outer streams respectively, have been used in the experiments. The structures of the triple flames have been compared for the different fuel combinations and equivalence ratios. The conditions under which triple flames exhibit oscillation have been identified. During the oscillation, the non-premixed flame and the outer lean premixed flame flicker strongly, while the inner rich premixed flame remains more or less stable. The flickering frequency has been evaluated through image processing and fast Fourier transform (FFT) of the average pixel intensity of the image frames. It is observed that, for all the fuel combinations, the frequency decreases with the increase in the outer equivalence ratio, while it is relatively invariant with the change in the inner equivalence ratio. However, an increase in the inner equivalence ratio affects the structure of the flame by increasing the heights of the inner premixed flame and non-premixed flame and also enlarges the yellow soot-laden zone at the tip of the inner flame. A scaling analysis of the oscillating flames has been performed based on the measured parameters, which show a variation of Strouhal number (St) with Richardson number (Ri) as St {proportional_to} Ri{sup 0.5}. The fuel type is found to have no influence on this correlation. (author)

  3. Finite rate chemistry and presumed PDF models for premixed turbulent combustion

    SciTech Connect

    Bray, K.N.C.; Swaminathan, N.; Champion, M.; Libby, P.A.

    2006-09-15

    The sensitivity of the prediction of mean reaction rates in turbulent premixed flames to presumed PDF shape is studied. Three different presumed PDF shapes are considered: (i) a beta function PDF, (ii) a twin delta function PDF, and (iii) a PDF based on unstrained laminar flame properties. The unstrained laminar flame has the same thermochemistry as the turbulent flame. Emphasis is placed on capturing the finite rate chemistry effects and obtaining a simple expression for the mean reaction rate. It is shown that, as the PDFs approach their bimodal limit, the mean reaction rate expressions obtained using the above three PDFs reduce to a common form. These expressions differ only in the numerical value of a multiplying factor. Predictions are compared with DNS data. Under the conditions of this comparison, the beta function and twin delta function PDFs lead to significant errors, while the PDF based on properties of an unstrained laminar flame gives good agreement with the DNS. (author)

  4. Local burning velocity in a Bunsen jet flame

    NASA Astrophysics Data System (ADS)

    García-Soriano, Gabriel; Castillo, José Luis; Higuera, Francisco J.; García-Ybarra, Pedro L.

    2012-11-01

    A PIV-based system has been set-up for the simultaneous measurement of the local burning velocity of premixed flames and the flame stretch due to the flame front curvature and the incoming flow strain rate. For moderately short jet flames, these measurements allow an indirect determination of the Markstein length, according to Clavin and Joulin (C-J) theory. For tall flames, the flame curvature becomes relatively large in a region around the tip where the C-J theory breaks down. However, our experiments confirm the appearance of a new linear relation between burning velocity and curvature at the flame tip. This relation defines a new proportionality factor which is probably associated to the evolution from rounded tips to slender tips when the jet velocity is increased.

  5. The effect of background turbulence on the propagation of large-scale flames

    NASA Astrophysics Data System (ADS)

    Matalon, Moshe

    2008-12-01

    This paper is based on an invited presentation at the Conference on Turbulent Mixing and Beyond held in the Abdus Salam International Center for Theoretical Physics, Trieste, Italy (August 2007). It consists of a summary of recent investigations aimed at understanding the nature and consequences of the Darrieus-Landau instability that is prominent in premixed combustion. It describes rigorous asymptotic methodologies used to simplify the propagation problem of multi-dimensional and time-dependent premixed flames in order to understand the nonlinear evolution of hydrodynamically unstable flames. In particular, it addresses the effect of background turbulent noise on the structure and propagation of large-scale flames.

  6. Study the effect of magnetic field on gaseous flames using digital speckle pattern interferometry

    NASA Astrophysics Data System (ADS)

    Kumar, Manoj; Agarwal, Shilpi; Kumar, Varun; Khan, Gufran S.; Shakher, Chandra

    2014-10-01

    An experimental investigation on the behavior of gaseous flames in the presence of magnetic field by using digital speckle pattern interferometry is presented. Premixed, partially premixed and diffusion flames generated by butane torch burner were exposed to the magnetic field of 0.35 Tesla. Phase has been extracted from a single DSPI fringe pattern by the application of Riesz transform and the monogenic signal and from which refractive index and the temperature were calculated. Experimental results show that the temperature and the width of the flames are increased under the influence of magnetic gradient.

  7. Flashback detection sensor for lean premix fuel nozzles

    DOEpatents

    Thornton, Jimmy Dean; Richards, George Alan; Straub, Douglas L.; Liese, Eric Arnold; Trader, Jr., John Lee; Fasching, George Edward

    2002-08-06

    A sensor for detecting the flame occurring during a flashback condition in the fuel nozzle of a lean premix combustion system is presented. The sensor comprises an electrically isolated flashback detection electrode and a guard electrode, both of which generate electrical fields extending to the walls of the combustion chamber and to the walls of the fuel nozzle. The sensor is positioned on the fuel nozzle center body at a location proximate the entrance to the combustion chamber of the gas turbine combustion system. The sensor provides 360.degree. detection of a flashback inside the fuel nozzle, by detecting the current conducted by the flame within a time frame that will prevent damage to the gas turbine combustion system caused by the flashback condition.

  8. Formation and Combustion of Smoke in Laminar Flames

    NASA Technical Reports Server (NTRS)

    Schalla, Rose L; Clark, Thomas P; Mcdonald, Glen E

    1954-01-01

    The nature and formation of smoke and its combustion were investigated. Smoke, which consist of tiny mesomorphous crystals tightly packed into popcorn-ball-like particles that agglomerate to give filaments, was found to contain about 5 percent of the hydrogen originally present in the fuel. Factors affecting smoke formation were studied in both diffusion flames and premixed Bunsen flames. It is suggested that smoking tendency increases with increasing stability of the carbon skeleton of the molecule, as determined by relative bond strength.

  9. Computations of turbulent lean premixed combustion using conditional moment closure

    NASA Astrophysics Data System (ADS)

    Amzin, Shokri; Swaminathan, Nedunchezhian

    2013-12-01

    Conditional Moment Closure (CMC) is a suitable method for predicting scalars such as carbon monoxide with slow chemical time scales in turbulent combustion. Although this method has been successfully applied to non-premixed combustion, its application to lean premixed combustion is rare. In this study the CMC method is used to compute piloted lean premixed combustion in a distributed combustion regime. The conditional scalar dissipation rate of the conditioning scalar, the progress variable, is closed using an algebraic model and turbulence is modelled using the standard k-ɛ model. The conditional mean reaction rate is closed using a first order CMC closure with the GRI-3.0 chemical mechanism to represent the chemical kinetics of methane oxidation. The PDF of the progress variable is obtained using a presumed shape with the Beta function. The computed results are compared with the experimental measurements and earlier computations using the transported PDF approach. The results show reasonable agreement with the experimental measurements and are consistent with the transported PDF computations. When the compounded effects of shear-turbulence and flame are strong, second order closures may be required for the CMC.

  10. Scaling of turbulent flame speed for expanding flames with Markstein diffusion considerations.

    PubMed

    Chaudhuri, Swetaprovo; Wu, Fujia; Law, Chung K

    2013-09-01

    In this paper we clarify the role of Markstein diffusivity, which is the product of the planar laminar flame speed and the Markstein length, on the turbulent flame speed and its scaling, based on experimental measurements on constant-pressure expanding turbulent flames. Turbulent flame propagation data are presented for premixed flames of mixtures of hydrogen, methane, ethylene, n-butane, and dimethyl ether with air, in near-isotropic turbulence in a dual-chamber, fan-stirred vessel. For each individual fuel-air mixture presented in this work and the recently published iso-octane data from Leeds, normalized turbulent flame speed data of individual fuel-air mixtures approximately follow a Re_{T,f}^{0.5} scaling, for which the average radius is the length scale and thermal diffusivity is the transport property of the turbulence Reynolds number. At a given Re_{T,f}^{}, it is experimentally observed that the normalized turbulent flame speed decreases with increasing Markstein number, which could be explained by considering Markstein diffusivity as the leading dissipation mechanism for the large wave number flame surface fluctuations. Consequently, by replacing thermal diffusivity with the Markstein diffusivity in the turbulence Reynolds number definition above, it is found that normalized turbulent flame speeds could be scaled by Re_{T,M}^{0.5} irrespective of the fuel, equivalence ratio, pressure, and turbulence intensity for positive Markstein number flames. PMID:24125342

  11. Scaling of turbulent flame speed for expanding flames with Markstein diffusion considerations.

    PubMed

    Chaudhuri, Swetaprovo; Wu, Fujia; Law, Chung K

    2013-09-01

    In this paper we clarify the role of Markstein diffusivity, which is the product of the planar laminar flame speed and the Markstein length, on the turbulent flame speed and its scaling, based on experimental measurements on constant-pressure expanding turbulent flames. Turbulent flame propagation data are presented for premixed flames of mixtures of hydrogen, methane, ethylene, n-butane, and dimethyl ether with air, in near-isotropic turbulence in a dual-chamber, fan-stirred vessel. For each individual fuel-air mixture presented in this work and the recently published iso-octane data from Leeds, normalized turbulent flame speed data of individual fuel-air mixtures approximately follow a Re_{T,f}^{0.5} scaling, for which the average radius is the length scale and thermal diffusivity is the transport property of the turbulence Reynolds number. At a given Re_{T,f}^{}, it is experimentally observed that the normalized turbulent flame speed decreases with increasing Markstein number, which could be explained by considering Markstein diffusivity as the leading dissipation mechanism for the large wave number flame surface fluctuations. Consequently, by replacing thermal diffusivity with the Markstein diffusivity in the turbulence Reynolds number definition above, it is found that normalized turbulent flame speeds could be scaled by Re_{T,M}^{0.5} irrespective of the fuel, equivalence ratio, pressure, and turbulence intensity for positive Markstein number flames.

  12. Scaling of turbulent flame speed for expanding flames with Markstein diffusion considerations

    NASA Astrophysics Data System (ADS)

    Chaudhuri, Swetaprovo; Wu, Fujia; Law, Chung K.

    2013-09-01

    In this paper we clarify the role of Markstein diffusivity, which is the product of the planar laminar flame speed and the Markstein length, on the turbulent flame speed and its scaling, based on experimental measurements on constant-pressure expanding turbulent flames. Turbulent flame propagation data are presented for premixed flames of mixtures of hydrogen, methane, ethylene, n-butane, and dimethyl ether with air, in near-isotropic turbulence in a dual-chamber, fan-stirred vessel. For each individual fuel-air mixture presented in this work and the recently published iso-octane data from Leeds, normalized turbulent flame speed data of individual fuel-air mixtures approximately follow a ReT,f0.5 scaling, for which the average radius is the length scale and thermal diffusivity is the transport property of the turbulence Reynolds number. At a given ReT,f, it is experimentally observed that the normalized turbulent flame speed decreases with increasing Markstein number, which could be explained by considering Markstein diffusivity as the leading dissipation mechanism for the large wave number flame surface fluctuations. Consequently, by replacing thermal diffusivity with the Markstein diffusivity in the turbulence Reynolds number definition above, it is found that normalized turbulent flame speeds could be scaled by ReT,M0.5 irrespective of the fuel, equivalence ratio, pressure, and turbulence intensity for positive Markstein number flames