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Sample records for 252cf spontaneous fission

  1. Bremsstrahlung emission of high energy accompanying spontaneous fission of {sup 252}Cf

    SciTech Connect

    Maydanyuk, S. P.; Olkhovsky, V. S.; Mandaglio, G.; Manganaro, M.; Fazio, G.; Giardina, G.

    2010-07-15

    The study of the bremsstrahlung photon emission accompanying fragments produced in the spontaneous fission of heavy nuclei by a fully quantum approach is presented for the first time. This kind of problem requires the knowledge of wave functions of the fissioning system leading to a wide distribution of couples of fragments that are the products of fission. With the aim of obtaining these wave functions, the interaction potential between the emitted fragment and residual nucleus is calculated by a standard approach. A new procedure was performed that allows an increase in the accuracy of calculations of radial integrals in the far asymptotic region and the achievement of the convenient convergence in calculations of the spectra. The total probability of the emitted photons in the spontaneous fission of {sup 252}Cf was calculated in such a way. We obtained good agreement between theory and experimental data up to 38 MeV for the bremsstrahlung spectrum of photons while the calculation of the total probability of photon emission accompanying fragments was performed up to an energy of 60 MeV. The analysis of contributions in the bremsstrahlung spectrum accompanying the emission of light, medium, and heavy fragments in the fission of {sup 252}Cf is presented.

  2. Relative Yields of 149-153Pr in Spontaneous Fission of 252Cf

    NASA Astrophysics Data System (ADS)

    Eldridge, Jonathan; Wang, Enhong; Hwang, J. K.; Hamilton, Joe; Ramayya, A. V.; Luo, Y. X.; Rasmussen, J. O.; Zhu, S. J.; Liu, S. H.; Ter-Akopian, G. M.; Oganessian, Yu. Ts.

    2013-10-01

    The relative yields of the fission partners of 149-153Pr, resulting from the spontaneous fission of 252Cf, were studied. This study was done by means of γ - γ - γ , and γ - γ - γ - γ coincidence data taken in 2000 by the multi-HPGe, Compton-suppressed, gamma detector array, Gammasphere, at Lawrence Berkeley National Lab. The coincidence data were analyzed by double- and triple-gating on transitions in 149-153Pr and obtaining the intensities of the 93-101Y transitions. For 150 , 151 , 152 , 153Pr the 3n channel was found to be the strongest. The 149Pr, however, was found to peak at the 4n channel. These results were used to verify the assignments of the level schemes of 151 , 152 , 153Pr. The data are found to be in agreement with Wahl's independent yield tables.

  3. Detailed Study of the Angular Correlations in the Prompt Neutron Emission in Spontaneous Fission of 252Cf

    NASA Astrophysics Data System (ADS)

    Kopatch, Yu.; Chietera, A.; Stuttgé, L.; Gönnenwein, F.; Mutterer, M.; Gagarski, A.; Guseva, I.; Chernysheva, E.; Dorvaux, O.; Hambsch, F.-J.; Hanappe, F.; Mezentseva, Z.; Telezhnikov, S.

    An experiment has been performed at IPHC Strasbourg, aimed at the detailed investigation of angular correlations in the neutron emission from spontaneous fission of 252Cf. Fission fragments were measured by the angle-sensitive double ionization chamber CODIS while neutrons were detected by a set of 60 DEMON scintillator counters. The main aim of the experiment is the observation of the correlation between the fragment spins and neutron emission anisotropy. Preliminary results, based on the Monte-Carlo simulations, as well as the preliminary analysis of the experimental data are shown.

  4. Analysis of linear energy transfers and quality factors of charged particles produced by spontaneous fission neutrons from 252Cf and 244Pu in the human body.

    PubMed

    Endo, Akira; Sato, Tatsuhiko

    2013-04-01

    Absorbed doses, linear energy transfers (LETs) and quality factors of secondary charged particles in organs and tissues, generated via the interactions of the spontaneous fission neutrons from (252)Cf and (244)Pu within the human body, were studied using the Particle and Heavy Ion Transport Code System (PHITS) coupled with the ICRP Reference Phantom. Both the absorbed doses and the quality factors in target organs generally decrease with increasing distance from the source organ. The analysis of LET distributions of secondary charged particles led to the identification of the relationship between LET spectra and target-source organ locations. A comparison between human body-averaged mean quality factors and fluence-averaged radiation weighting factors showed that the current numerical conventions for the radiation weighting factors of neutrons, updated in ICRP103, and the quality factors for internal exposure are valid.

  5. Characterization of neutron fields from bare and heavy water moderated (252)Cf spontaneous fission source using Bonner Sphere Spectrometer.

    PubMed

    Atanackovic, Jovica; Yonkeu, Andre; Dubeau, Jacques; Witharana, Sampath Hakmana; Priest, Nicholas

    2015-05-01

    In this work a calibrated Bonner Sphere Spectrometer (BSS), together with ISO shadow cones, was used to quantify the total and scattered components of bare and heavy water moderated (252)Cf neutron fields. All measurements were performed with a BSS that was calibrated at the National Physical Laboratory (NPL), Teddington, UK, which is a global primary standard laboratory and world-leading facility for neutron metrology and neutron instruments calibration. The fields were characterized for source-spectrometer distances of 80, 100, 150 and 200cm; and at heights of 103 and 200cm from the facility floor. As expected, the scattered contribution was greatest at the farthest distance from the source and closer to the floor. Hence, at a distance of 200cm and a height of 103cm, the scatter added to the direct field up to 162% of the total neutron fluence and up to 61% of the ambient dose equivalent, while at the same distance and height of 200cm above the floor, these values were up to 146% and 52%, respectively. In the case of heavy water moderated (252)Cf neutron fields, a shadow cone subtraction technique could not be implemented, however Monte Carlo simulations were utilized in order to differentiate between the direct and scatter components of the neutron fields. In this case, at a source-detector distance of 200cm and a height of 103cm, the scatter added to the direct field up to 148% of the total neutron fluence and up to 45% of the ambient dose equivalent, while at the same distance and a height of 200cm above the floor, these values were up to 134% and 42%, respectively.

  6. Comparison of fission modes in {sup 252}Cf, {sup 257}Fm, and {sup 260}Md

    SciTech Connect

    Aarle, J. van; Siemon, K.; Patzelt, P.; Wild, J. F.; Lougheed, R. W.; Westmeier, W.

    1998-10-26

    Although the spontaneous-fission properties of heavy actinides have been studied for well over 35 years, many interesting and informative details continue to come into light. During the last decade, the spontaneous fission of {sup 252}Cf, {sup 257}Fm and {sup 260}Md has been extensively investigated at the Philipps University of Marburg, by means of a gadolinium-doped liquid scintillation tank for neutron counting and surface barrier detectors for fission fragment detection. The three nuclides represent the transition from the well-known asymmetric fission yield distribution, as it is characteristic for {sup 252}Cf, to a much more symmetrical one, found in the fission of {sup 260}Md. Therefore, trends in the dynamical changes of fission properties have been derived from these studies. For the spontaneous fission of {sup 252}Cf and {sup 260}Md, it was already shown that different fission modes, as proposed by theoretical calculations of Brosa et al. (5), could be separated, using the correlation between the neutrons emitted in a fission event and both the observed fission-fragment mass and the total kinetic energy (1, 2). In the case of {sup 257}Fm, no theoretical calculations for fission modes exist. However, from the fission properties of the two surrounding actinides, one can expect at least three different fission modes, namely two 'standard' and the 'supershort' mode. In this paper, results from the recent {sup 257}Fm experiment will be presented and compared to systematics extracted from the fission properties of other heavy actinides.

  7. Comparison of fission modes in {sup 252}Cf, {sup 257}Fm, and {sup 260}Md

    SciTech Connect

    van Aarle, J.; Siemon, K.; Patzelt, P.; Wild, J.F.; Lougheed, R.W.; Westmeier, W.

    1998-10-01

    Although the spontaneous-fission properties of heavy actinides have been studied for well over 35 years, many interesting and informative details continue to come into light. During the last decade, the spontaneous fission of {sup 252}Cf, {sup 257}Fm and {sup 260}Md has been extensively investigated at the Philipps University of Marburg (1{endash}4), by means of a gadolinium-doped liquid scintillation tank for neutron counting and surface barrier detectors for fission fragment detection. The three nuclides represent the transition from the well-known asymmetric fission yield distribution, as it is characteristic for {sup 252}Cf, to a much more symmetrical one, found in the fission of {sup 260}Md. Therefore, trends in the dynamical changes of fission properties have been derived from these studies. For the spontaneous fission of {sup 252}Cf and {sup 260}Md, it was already shown that different fission modes, as proposed by theoretical calculations of Brosa et al. (5), could be separated, using the correlation between the neutrons emitted in a fission event and both the observed fission-fragment mass and the total kinetic energy (1, 2). In the case of {sup 257}Fm, no theoretical calculations for fission modes exist. However, from the fission properties of the two surrounding actinides, one can expect at least three different fission modes, namely two {open_quotes}standard{close_quotes} and the {open_quotes}supershort{close_quotes} mode. In this paper, results from the recent {sup 257}Fm experiment will be presented and compared to systematics extracted from the fission properties of other heavy actinides. {copyright} {ital 1998 American Institute of Physics.}

  8. Microscopic cold fission yields of {sup 252}Cf

    SciTech Connect

    Mirea, M.; Delion, D. S.; Sandulescu, A.

    2010-04-15

    We show that the sharp maximum corresponding to {sup 107}Mo in the fragment distribution of the {sup 252}Cf cold fission is actually a Sn-like radioactivity, similar to other decay processes in which magic nuclei are involved, namely alpha decay and heavy cluster emission, also called Pb-like radioactivity. It turns out that the mass asymmetry degree of freedom has a key role in connecting initial Sn with the final Mo isotopes along the fission path. We investigate the cold rearrangement of nucleons within the framework of the two-center shell model in order to compute the cold valleys in the charge equilibrated fragmentation potential. The fission yields are estimated by using the semiclassical penetration approach. We consider 5 degrees of freedom, namely the interfragment distance, the shapes of fragments, the neck parameter, and mass asymmetry. We found an isomeric minimum between the internal and external barriers. It turns out that the inner cold valley of the total potential energy is connected to the doubly magic isotope {sup 132}Sn.

  9. Identification of high spin states in {sup 134}I from {sup 252}Cf fission

    SciTech Connect

    Liu, S. H.; Hamilton, J. H.; Ramayya, A. V.; Hwang, J. K.; Daniel, A. V.; Ter-Akopian, G. M.; Luo, Y. X.; Rasmussen, J. O.; Zhu, S. J.; Ma, W. C.

    2009-06-15

    High spin states in {sup 134}I were identified for the first time based on measurements of prompt {gamma} rays from the spontaneous fission of {sup 252}Cf at Gammasphere. Five excited levels with five deexciting transitions were observed. The mass number was assigned based on the intensity of transitions in the complementary Rh fragments. Angular correlations for the first two transitions in {sup 134}I and for high spin states in {sup 133,135,136}I were performed, but were not sufficient to firmly assign the spins and parities in {sup 134}I.

  10. True ternary fission, the collinear cluster tripartition (CCT) of {sup 252}Cf

    SciTech Connect

    Oertzen, W. von; Pyatkov, Y. V.; Kamanin, D.

    2012-10-20

    In systematic work over the last decade (see Pyatkov et al. [12] and refs therein), the ternary fission decay of heavy nuclei, in {sup 235}U(n,fff) and {sup 252}Cf(sf) has been studied in a collinear geometry. The name used for this process is (CCT), with three fragments of similar size in a collinear decay, it is the true ternary fission. This decay has been observed in spontaneous fission as well as in a neutron induced reaction. The measurements are based on different experimental set-ups, with binary coincidences containing TOF and energy determinations. With two detector telescopes placed at 180 Degree-Sign , the measurements of masses and energies of each of the registered two fragments, give complete kinematic solutions. Thus the missing mass events in binary coincidences can be determined, these events are obtained by blocking one of the lighter fragments on a structure in front of the detectors. The relatively high yield of CCT (more than 10{sup -3} per binary fission) is explained. It is due to the favourable Q-values (more positive than for binary) and the large phase space of the ternary CCT-decay, dominated by three (magic) clusters: e.g. isotopes of Sn, Ca and Ni, {sup 132}Sn+{sup 50}Ca+{sup 70}Ni. It is shown that the collinear (prolate) geometry has the favoured potential energy relative to the oblate shapes. The ternary fission is considered to be a sequential process. With this assumption the kinetic energies of the fragments have been calculated by Vijay et al.. The third fragments have very low kinetic energies (below 20 MeV) and have thus escaped their detection in previous work on 'ternary fission', where in addition an oblate shape and a triangle for the momentum vectors have been assumed.

  11. True ternary fission, the collinear cluster tripartition (CCT) of 252Cf

    NASA Astrophysics Data System (ADS)

    von Oertzen, W.; Pyatkov, Y. V.; Kamanin, D.

    2012-10-01

    In systematic work over the last decade (see Pyatkov et al. [12] and refs therein), the ternary fission decay of heavy nuclei, in 235U(n,fff) and 252Cf(sf) has been studied in a collinear geometry. The name used for this process is (CCT), with three fragments of similar size in a collinear decay, it is the true ternary fission. This decay has been observed in spontaneous fission as well as in a neutron induced reaction. The measurements are based on different experimental set-ups, with binary coincidences containing TOF and energy determinations. With two detector telescopes placed at 180°, the measurements of masses and energies of each of the registered two fragments, give complete kinematic solutions. Thus the missing mass events in binary coincidences can be determined, these events are obtained by blocking one of the lighter fragments on a structure in front of the detectors. The relatively high yield of CCT (more than 10-3 per binary fission) is explained. It is due to the favourable Q-values (more positive than for binary) and the large phase space of the ternary CCT-decay, dominated by three (magic) clusters: e.g. isotopes of Sn, Ca and Ni, 132Sn+50Ca+70Ni. It is shown that the collinear (prolate) geometry has the favoured potential energy relative to the oblate shapes. The ternary fission is considered to be a sequential process. With this assumption the kinetic energies of the fragments have been calculated by Vijay et al. [1]. The third fragments have very low kinetic energies (below 20 MeV) and have thus escaped their detection in previous work on "ternary fission", where in addition an oblate shape and a triangle for the momentum vectors have been assumed.

  12. 252Cf fission-neutron spectrum using a simplified time-of-flight setup: An advanced teaching laboratory experiment

    NASA Astrophysics Data System (ADS)

    Becchetti, F. D.; Febbraro, M.; Torres-Isea, R.; Ojaruega, M.; Baum, L.

    2013-02-01

    The removal of PuBe and AmBe neutron sources from many university teaching laboratories (due to heightened security issues) has often left a void in teaching various aspects of neutron physics. We have recently replaced such sources with sealed 252Cf oil-well logging sources (nominal 10-100 μCi), and developed several experiments using them as neutron sources. This includes a fission-neutron time-of-flight experiment using plastic scintillators, which utilizes the prompt γ rays emitted in 252Cf spontaneous fission as a fast timing start signal. The experiment can be performed with conventional nuclear instrumentation and a 1-D multi-channel pulse-height analyzer, available in most advanced teaching laboratories. Alternatively, a more sophisticated experiment using liquid scintillators and n/γ pulse-shape discrimination can be performed. Several other experiments using these neutron sources are also feasible. The experiments can introduce students to the problem of detecting the dark matter thought to dominate the universe and to the techniques used to detect contraband fissionable nuclear materials.

  13. Radioactive Beams from 252Cf Fission Using a Gas Catcher and an ECR Charge Breeder at ATLAS

    SciTech Connect

    Savard, Guy; Pardo, Richard C.; Moore, E. Frank; Hecht, Adam A.; Baker, Sam

    2005-03-15

    A proposed upgrade to the radioactive beam capability of the ATLAS facility has been proposed using 252Cf fission fragments thermalized and collected into a low-energy particle beam using a helium gas catcher. In order to reaccelerate these beams the ATLAS ECR-I will be reconfigured as a charge breeder source. A 1Ci 252Cf source is expected to provide sufficient yield to deliver beams of up to {approx}103 far from stability ions per second on target. A brief facility description and the expected performance information are provided in this report.

  14. Structures of the neutron-rich nuclei observed in fission of {sup 252}Cf

    SciTech Connect

    Ramayya, A. V.; Hamilton, J. H.; Goodin, C. J.; Brewer, N. T.; Hwang, J. K.; Luo, Y. X.; Liu, S. H.; Stone, N. J.; Daniel, A. V.; Zhu, S. J.

    2014-08-14

    Analysis of high statistics triple coincidence fission γ data from {sup 252}Cf at Gammasphere including angular correlations yielded well-expanded high-spin level schemes with more complete and reliable spin/parity assignments for {sup 82}Ge, {sup 118,120,122}Cd and {sup 114,115}Rh. Both the quasi-particle/hole couplings and quasi-rotational degrees of freedom are implied to play roles in these Cd isotopes. Evidence for triaxial shapes and octupole components in the Cd isotopes is presented. These Cd isotopes may have triaxial deformations. High-spin level schemes of {sup 114,115}Rh have been established for the first time. The existence of a relatively large signature splitting and an yrare band shows typical features of a triaxially deformed nucleus. Possible excited deformed rotational bands are observed, for the first time, in {sup 82}Ge. From the multipole mixing ratio measurement, the ground state configurations of {sup 109,111}Ru, as well as excited states in {sup 103,107}Mo and {sup 111}Ru were determined.

  15. Status of the electron cyclotron resonance charge breeder for the {sup 252}Cf fission source project at ATLAS

    SciTech Connect

    Vondrasek, R. C.; Scott, R.; Carr, J.; Pardo, R. C.

    2008-02-15

    The construction of the Californium Rare Ion Breeder Upgrade, a new radioactive beam facility for the Argonne tandem linac accelerator system (ATLAS), is in progress. The facility will use fission fragments from a 1 Ci {sup 252}Cf source, thermalized and collected into a low-energy particle beam by a helium gas catcher. In order to reaccelerate these beams, the existing ATLAS ECR1 ion source has been redesigned to function as a charge breeder source. The design features, initial results, and status of this charge breeder configuration are presented.

  16. The content of 250Cf and 248Cm in 252Cf neutron sources and the effect on the neutron emission rate.

    PubMed

    Roberts, N J; Jones, L N

    2007-01-01

    One of the most common radionuclide neutron sources used for the calibration of detectors is (252)Cf. However, these sources also contain (250)Cf, which is present in the material from which the sources are made, and (248)Cm, which is formed as the daughter of (252)Cf via alpha-decay. Both decay by spontaneous fission with longer half-lives than (252)Cf. Consequently, as the source becomes older, the emission rate does not follow the decay curve of (252)Cf. Fits have been made to emission rate measurements of (252)Cf sources at NPL spanning over 30 y to deduce their (250)Cf and (248)Cm content. The emission rate of a source can be significantly underestimated if the presence of (250)Cf and (248)Cm is not taken into account, and this has been investigated for a typical (252)Cf source. The importance of this problem to other calibration laboratories and users of (252)Cf sources is emphasised.

  17. True ternary fission, the collinear decay into fragments of similar size in the 252Cf(sf) and 235U(nth, f) reactions

    NASA Astrophysics Data System (ADS)

    von Oertzen, W.; Nasirov, A. K.

    2014-06-01

    The collinear cluster decay in 252Cf(sf, fff), with three cluster fragments of different masses (e.g. 132Sn, 52-48Ca, 68-72Ni), which has been observed by the FOBOS group in JINR, has established a new decay mode of heavy nuclei, the collinear cluster tripartition (CCT). The same type of ternary fission decay has been observed in the reaction 235U(nth, fff). This kind of “true ternary fission” of heavy nuclei has been predicted many times in theoretical works during the last decades. In the present note we discuss true ternary fission (TFFF) into three nuclei of almost equal size (e.g. Z=98→Zi=32, 34, 32) in the same systems. The possible fission channels are predicted from potential-energy (PES) calculations. These PES's show pronounced minima for several ternary fragmentation decays, e.g. for 252Cf(sf) and for 235U(nth, f). They suggest the existence of a variety of collinear ternary fission modes. The TFFF-decays chosen in this letter have very similar dynamical features as the previously observed collinear CCT-decays. The data obtained in the above mentioned experiments allow us to extract the yield for these TFFF-decays in both systems by using specific gates on the measured parameters. These yields are a few 1.0ṡ10-6/(binary fission).

  18. Results with the electron cyclotron resonance charge breeder for the 252Cf fission source project (Californium Rare Ion Breeder Upgrade) at Argonne Tandem Linac Accelerator System.

    PubMed

    Vondrasek, R; Kondrashev, S; Pardo, R; Scott, R; Zinkann, G P

    2010-02-01

    The construction of the Californium Rare Ion Breeder Upgrade, a new radioactive beam facility for the Argonne Tandem Linac Accelerator System (ATLAS), is nearing completion. The facility will use fission fragments from a 1 Ci (252)Cf source; thermalized and collected into a low-energy particle beam by a helium gas catcher. In order to reaccelerate these beams, an existing ATLAS electron cyclotron resonance (ECR) ion source was redesigned to function as an ECR charge breeder. Thus far, the charge breeder has been tested with stable beams of rubidium and cesium achieving charge breeding efficiencies of 9.7% into (85)Rb(17+) and 2.9% into (133)Cs(20+).

  19. Results with the electron cyclotron resonance charge breeder for the {sup 252}Cf fission source project (Californium Rare Ion Breeder Upgrade) at Argonne Tandem Linac Accelerator System

    SciTech Connect

    Vondrasek, R.; Kondrashev, S.; Pardo, R.; Scott, R.; Zinkann, G. P.

    2010-02-15

    The construction of the Californium Rare Ion Breeder Upgrade, a new radioactive beam facility for the Argonne Tandem Linac Accelerator System (ATLAS), is nearing completion. The facility will use fission fragments from a 1 Ci {sup 252}Cf source; thermalized and collected into a low-energy particle beam by a helium gas catcher. In order to reaccelerate these beams, an existing ATLAS electron cyclotron resonance (ECR) ion source was redesigned to function as an ECR charge breeder. Thus far, the charge breeder has been tested with stable beams of rubidium and cesium achieving charge breeding efficiencies of 9.7% into {sup 85}Rb{sup 17+} and 2.9% into {sup 133}Cs{sup 20+}.

  20. Spontaneous Fission

    DOE R&D Accomplishments Database

    Segre, Emilio

    1950-11-22

    The first attempt to discover spontaneous fission in uranium was made by [Willard] Libby, who, however, failed to detect it on account of the smallness of effect. In 1940, [K. A.] Petrzhak and [G. N.] Flerov, using more sensitive methods, discovered spontaneous fission in uranium and gave some rough estimates of the spontaneous fission decay constant of this substance. Subsequently, extensive experimental work on the subject has been performed by several investigators and will be quoted in the various sections. [N.] Bohr and [A.] Wheeler have given a theory of the effect based on the usual ideas of penetration of potential barriers. On this project spontaneous fission has been studied for the past several years in an effort to obtain a complete picture of the phenomenon. For this purpose the spontaneous fission decay constants {lambda} have been measured for separated isotopes of the heavy elements wherever possible. Moreover, the number {nu} of neutrons emitted per fission has been measured wherever feasible, and other characteristics of the spontaneous fission process have been studied. This report summarizes the spontaneous fission work done at Los Alamos up to January 1, 1945. A chronological record of the work is contained in the Los Alamos monthly reports.

  1. Spontaneous fission

    SciTech Connect

    Hoffman, D.C.

    1993-09-01

    The spontaneous fission (SF) of the heaviest actinides and the transactinides is of particular interest because of the dramatic changes in properties observed in the region of the heavy fermion isotopes and for still heavier elements. The existing experimental information on SF properties including half-life systematics, fragment kinetic-energy and mass-yield distributions, prompt neutron emission, and gamma emission will be reviewed. Possibility for extending studies of SF properties to other regions are considered and the potential for obtaining additional information about low-energy fission properties is discussed.

  2. Graphite moderated (252)Cf source.

    PubMed

    Sajo-Bohus, Laszlo; Barros, Haydn; Greaves, Eduardo D; Vega-Carrillo, Hector Rene

    2015-06-01

    The Thorium molten-salt reactor is an attractive and affordable nuclear power option for developing countries with insufficient infrastructure and limited technological capability. In the aim of personnel training and experience gathering at the Universidad Simon Bolivar there is in progress a project of developing a subcritical thorium liquid-fuel reactor. The neutron source to run this subcritical reactor is a (252)Cf source and the reactor will use high-purity graphite as moderator. Using the MCNP5 code the neutron spectra of the (252)Cf in the center of the graphite moderator has been estimated along the channel where the liquid thorium salt will be inserted; also the ambient dose equivalent due to the source has been determined around the moderator.

  3. Multimodal fission and neutron evaporation

    SciTech Connect

    Brosa, U.

    1988-10-01

    The average multiplicities nu-bar(A) of prompt neutrons emitted in the spontaneous fission of /sup 252/Cf and /sup 258/Fm are derived. Two new features are predicted: A simple sawtooth for /sup 258/Fm and a triple one for /sup 252/Cf. Experiments to check these predictions should be feasible now.

  4. A New Facility For Non-Destructive Assay With A Time-Tagged {sup 252}Cf Source

    SciTech Connect

    Stevanato, L.; Caldogno, M.; Hao, Xin; Dima, R.; Fabris, D.; Nebbia, G.; Lunardon, M.; Moretto, S.; Pesente, S.; Viesti, G.; Sajo-Bohus, L.

    2011-06-01

    A new facility for Non-Destructive Assay based on a time-tagged {sup 252}Cf spontaneous fission source is now in operation at the Padova University. The system is designed to analyze samples with dimensions on the order of 20x20 cm{sup 2}, the material recognition being obtained by measuring simultaneously transmission of neutrons and gamma rays as a function of energy.

  5. Absolute measurement of anti. nu. /sub p/ for /sup 252/Cf using the ORNL large liquid scintillator neutron detector

    SciTech Connect

    Spencer, R.R.; Gwin, R.; Ingle, R.

    1981-08-01

    The ORNL large liquid scintillator detector was used in a precise determination of anti ..nu../sub p/, the number of neutrons emitted promptly, for spontaneous fission of /sup 252/Cf. Measurements of the detector efficiency over a broad energy region were made by means of a proton-recoil technique employing the ORELA white neutron source. Monte Carlo calculation of the detector efficiency for a spectrum representative of /sup 252/Cf fission neutrons was calibrated with these elaborate measurements. The unusually flat response of the neutron detector resulted in elimination of several known sources of error. Experimental measurement was coupled with calculational methods to correct for other known errors. These measurements lead to an unusually small estimated uncertainty of 0.2% in the value obtained, anti ..nu../sub p/ = 3.773 +- 0.007.

  6. Measurement and calculation of the emission anisotropy of an X1 252Cf neutron source.

    PubMed

    Hawkes, N P; Freedman, R; Tagziria, H; Thomas, D J

    2007-01-01

    The authors have measured the emission anisotropy from a (252)Cf spontaneous fission neutron source in an X1 encapsulation. The measurements were made in a large low-scatter laboratory using a long counter, and data were taken at angles varying in 10 degrees steps from 0 degrees to 180 degrees relative to the cylindrical axis of the source. Corrections were made for room scatter, loss of neutrons due to air scatter and detector dead time. Calculations corresponding to these measurements were subsequently carried out using the two Monte Carlo codes MCNP and MCBEND, and the results are compared with the measurements and with each other.

  7. Spontaneous fission of the heaviest elements

    SciTech Connect

    Hoffman, D.C.

    1989-04-01

    Although spontaneous fission was discovered in /sup 238/U in 1940, detailed studies of the process were first made possible in the 1960's with the availability of milligram quantities of /sup 252/Cf. The advent of solid-state detectors made it possible to perform measurements of coincident fission fragments from even very short-lived spontaneous fission activities or those available in only very small quantities. Until 1971 it was believed that the main features of the mass and kinetic-energy distributions were essentially the same as those for thermal neutron-induced fission and that all low-energy fission proceeded via asymmetric mass division with total kinetic energies which could be derived by linear extrapolation from those of lighter elements. In 1971, measurements of /sup 257/Fm showed an increase in symmetric mass division with anomalously high TKE's. Subsequent experiments showed that in /sup 258/Fm and /sup 259/Fm, the most probable mass split was symmetric with very high total kinetic energy. Measurements for the heavier elements have shown symmetric mass distributions with both high and low total kinetic energies. Recent results for spontaneous fission properties of the heaviest elements are reviewed and compared with theory. 31 refs., 8 figs., 1 tab.

  8. Results with the electron cyclotron resonance charge breeder for the 252Cf fission source project (Californium Rare Ion Breeder Upgrade) at Argonne Tandem Linac Accelerator System

    NASA Astrophysics Data System (ADS)

    Vondrasek, R.; Kondrashev, S.; Pardo, R.; Scott, R.; Zinkann, G. P.

    2010-02-01

    The construction of the Californium Rare Ion Breeder Upgrade, a new radioactive beam facility for the Argonne Tandem Linac Accelerator System (ATLAS), is nearing completion. The facility will use fission fragments from a 1 Ci C252f source; thermalized and collected into a low-energy particle beam by a helium gas catcher. In order to reaccelerate these beams, an existing ATLAS electron cyclotron resonance (ECR) ion source was redesigned to function as an ECR charge breeder. Thus far, the charge breeder has been tested with stable beams of rubidium and cesium achieving charge breeding efficiencies of 9.7% into R85b17+ and 2.9% into C133s20+.

  9. 252Cf spectrum-averaged cross section for the 63Cu(n, p)63Ni reaction

    NASA Astrophysics Data System (ADS)

    Imamura, M.; Shibata, T.; Shibata, S.; Ohkubo, T.; Satoh, S.; Nogawa, N.

    1999-01-01

    The 63Ni produced by the 63Cu(n, p)63Ni reaction provides a unique measure to estimate the fast-neutron fluence of the Hiroshima/Nagasaki atomic bomb. In the similarity of the fission neutron spectrum of 252Cf to that of 235U, we have measured activation cross sections of the 63Cu(n, p)63Ni reaction averaged for the 252Cf fission spectrum.

  10. Biomodal spontaneous fission

    SciTech Connect

    Hulet, E.K. )

    1989-09-26

    Investigations of mass and kinetic-energy distributions from spontaneous fission have been extended in recent years to an isotope of element 104 and, for half-lives, to an isotope of element 108. The results have been surprising in that spontaneous fission half-lives have turned out to be much longer than expected and mass and kinetic- energy distributions were found to abruptly shift away from those of the lighter actinides, showing two modes of fission. These new developments have caused a re-evaluation of our understanding of the fission process, bringing an even deeper appreciation of the role played by nuclear shell effects upon spontaneous fission properties. 16 refs., 10 figs.

  11. Neutron angular distribution in plutonium-240 spontaneous fission

    NASA Astrophysics Data System (ADS)

    Marcath, Matthew J.; Shin, Tony H.; Clarke, Shaun D.; Peerani, Paolo; Pozzi, Sara A.

    2016-09-01

    Nuclear safeguards applications require accurate fission models that exhibit prompt neutron anisotropy. In the laboratory reference frame, an anisotropic neutron angular distribution is observed because prompt fission neutrons carry momentum from fully accelerated fission fragments. A liquid organic scintillation detector array was used with pulse shape discrimination techniques to produce neutron-neutron cross-correlation time distributions and angular distributions from spontaneous fission in a 252Cf, a 0.84 g 240Pueff metal, and a 1.63 g 240Pueff metal sample. The effect of cross-talk, estimated with MCNPX-PoliMi simulations, is removed from neutron-neutron coincidences as a function of the angle between detector pairs. Fewer coincidences were observed at detector angles near 90°, relative to higher and lower detector angles. As light output threshold increases, the observed anisotropy increases due to spectral effects arising from fission fragment momentum transfer to emitted neutrons. Stronger anisotropy was observed in Cf-252 spontaneous fission prompt neutrons than in Pu-240 neutrons.

  12. Dynamics and energetics of a /sup 251/Cf-/sup 252/Cf power system

    SciTech Connect

    Harms, A.A. ); Cripps, G. )

    1988-06-01

    A combination fission-radioisotope compact power system involving the synergistic interaction of /sup 251/Cf and /sup 252/Cf is considered. Based on a nonlinear point kinetics formulation of the coupled reactions combined with the parametric incorporation of design and operational variables, it is shown that a stable autonomous power mode is readily attainable. This system appears particularly suitable for very long-life unattended operation for space and terrestrial applications.

  13. Neutron multiplicities in spontaneous fission and nuclear structure studies

    SciTech Connect

    Hamilton, J.H.; Kormicki, J.; Lu, Q.

    1993-12-31

    New insights into the fission process can be gained by better quantitative knowledge of how the energy released in fission is distributed between the kinetic energy of the two fragments, the excitation energy of the two fragments and the number of neutrons emitted. Studies of prompt gamma-rays emitted in spontaneous fission (SF) with large arrays of Compton suppressed Ge detector arrays are providing new quantitative answers to longstanding questions concerning fission as well as new insights into the structure of neutron-rich nuclei. For the first time the triple gamma coincidence technique was employed in spontaneous fission studies. Studies of SF of {sup 252}Cf and {sup 242}Pu have been carried out. These {gamma}-{gamma}-{gamma} data provide powerful ways to identify uniquely gamma rays from a particular nucleus in the very complex gamma-ray spectra given off by the over 100 different nuclei produced. The emphasis of this paper is on the first quantitative measurements of the multiplicities of the neutrons emitted in SF and the energy levels populated in the fragments. Indeed, in the break up into Mo-Ba pairs, we have identified for the first time fragments associated with from zero up to ten neutrons emitted and observed the excited energy states populated in these nuclei. The zero neutron emission pairs like {sup 104}Mo- {sup 148}Ba, {sup 106}Mo- {sup 146}Ba and {sup 104}Zr- {sup 148}Ce observed in this work are particularly interesting because they represent a type of cold fission or a new mode of cluster radioactivity as proposed by Greiner, Sandulescu and co-workers. These data provide new insights into the processes of cluster radioactivity and cold fission.

  14. ANISOTROPY FACTORS FOR A 252Cf SOURCE

    SciTech Connect

    Veinot, K. G.; Bogard, James S

    2009-01-01

    A new 252Cf source has been procured for use at the Dosimetry Applications and Research (DOSAR) facility at the Oak Ridge National Laboratory (ORNL). This source was encapsulated by the Californium Facility at ORNL, however, the encapsulation differs from previous designs designated as SR-Cf-100. The new encapsulation, designated SR-Cf-3000, has a similar cylindrical radius to the previous generation, but is 1.6 cm longer. Since the encapsulation geometries differ the amount of internal scattering of neutrons will also differ leading to changes in anisotropy factors between the two designs. Additionally, the different encapsulations will affect the absorbed dose and dose equivalent delivered per neutron emitted by the source since both the quantity and energy distribution of the emitted neutrons will vary with irradiation angle. This work presents the fluence anisotropy factors for the SR-Cf-3000 series encapsulation as well as absorbed dose and dose equivalent values calculated for various angles of irradiation. The fluence anisotropy factors vary from a maximum of 1.037 to a minimum of 0.641 for irradiation angles perpendicular and parallel to the source axis, respectively. Anisotropy in absorbed dose varied from a maximum of 1.033 to a minimum of 0.676 while anisotropy of dose equivalent varied from 1.035 to 0.657.

  15. Student Experiments in Spontaneous Fission.

    ERIC Educational Resources Information Center

    Becchetti, F. D.; Ying, J. S.

    1981-01-01

    Advanced undergraduate experiments utilizing a commercially available, thin spontaneous fission source are described, including studies of the energy and mass distribution of the fission fragments and their energy and angular correlation. The experiments provide a useful introduction to fission, nuclear mass equations, heavy-ion physics, and…

  16. Attributes and templates from active measurements with {sup 252}Cf

    SciTech Connect

    Mihalczo, J.T.; Mattingly, J.K.

    2000-02-01

    Active neutron interrogation is useful for the detection of shielded HEU and could also be used for Pu. In an active technique, fissile material is stimulated by an external neutron source to produce fission with the emanation of neutrons and gamma rays. The time distribution of particles leaving the fissile material is measured with respect to the source emission in a variety of ways. A variety of accelerator and radioactive sources can be used. Active interrogation of nuclear weapons/components can be used in two ways: template matching or attribute estimation. Template matching compares radiation signatures with known reference signatures and for treaty applications has the problem of authentication of the reference signatures along with storage and retrieval of templates. Attribute estimation determines, for example, the fissile mass from various features of the radiation signatures and does not require storage of radiation signatures but does require calibration, which can be repeated as necessary. A nuclear materials identification system (NMIS) has been in use at the Oak Ridge Y-12 Plant for verification of weapons components being received and in storage by template matching and has been used with calibrations for attribute (fissile mass) estimation for HEU metal. NMIS employs a {sup 252}Cf source of low intensity (< 2 x 10{sup 6} n/sec) such that the dose at 1 m is approximately twice that on a commercial airline at altitude. The use of such a source presents no significant safety concerns either for personnel or nuclear explosive safety, and has been approved for use at the Pantex Plant on fully assembled weapons systems.

  17. Spontaneous Fission: A Kinetic Approach

    SciTech Connect

    Bonasera, A.; Iwamoto, A.; Bonasera, A.

    1997-01-01

    We present an attempt towards the many-body description of spontaneous fission based on the semiclassical Vlasov equation and the Feynman path integral method. We define suitable collective variables from the Vlasov solution and use the imaginary time technique for the dynamics below the Coulomb barrier. We demonstrate (1) the stability of the Vlasov solution, (2) the ability of this model to calculate the basic features of the whole spontaneous fission process, (3) the sensitivity of the dynamics below the barrier to the mean field potential, and (4) the important role of collective excitations and of particle emission during the fission process. {copyright} {ital 1997} {ital The American Physical Society}

  18. The SPIDER fission fragment spectrometer for fission product yield measurements

    DOE PAGES

    Meierbachtol, K.; Tovesson, F.; Shields, D.; Arnold, C.; Blakeley, R.; Bredeweg, T.; Devlin, M.; Hecht, A. A.; Heffern, L. E.; Jorgenson, J.; et al

    2015-04-01

    The SPectrometer for Ion DEtermination in fission Research (SPIDER) developed for measuring mass yield distributions of fission products from spontaneous and neutron-induced fission. The 2E–2v method of measuring the kinetic energy (E) and velocity (v) of both outgoing fission products utilized, with the goal of measuring the mass of the fission products with an average resolution of 1 atomic mass unit (amu). The SPIDER instrument, consisting of detector components for time-of-flight, trajectory, and energy measurements, assembled and tested using 229Th and 252Cf radioactive decay sources. For commissioning, the fully assembled system measured fission products from spontaneous fission of 252Cf. Finally,more » individual measurement resolutions were met for time-of-flight (250 ps FWHM), spacial resolution (2 mm FHWM), and energy (92 keV FWHM for 8.376 MeV). These mass yield results measured from 252Cf spontaneous fission products are reported from an E–v measurement.« less

  19. Reactor production of sup 252 Cf and transcurium isotopes

    SciTech Connect

    Alexander, C.W.; Halperin, J.; Walker, R.L.; Bigelow, J.E.

    1990-01-01

    Berkelium, californium, einsteinium, and fermium are currently produced in the High Flux Isotope Reactor (HFIR) and recovered in the Radiochemical Engineering Development Center (REDC) at the Oak Ridge National Laboratory (ORNL). All the isotopes are used for research. In addition, {sup 252}Cf, {sup 253}Es, and {sup 255}Fm have been considered or are used for industrial or medical applications. ORNL is the sole producer of these transcurium isotopes in the western world. A wide range of actinide samples were irradiated in special test assemblies at the Fast Flux Test Facility (FFTF) at Hanford, Washington. The purpose of the experiments was to evaluate the usefulness of the two-group flux model for transmutations in the special assemblies with an eventual goal of determining the feasibility of producing macro amounts of transcurium isotopes in the FFTF. Preliminary results from the production of {sup 254g}Es from {sup 252}Cf will be discussed. 14 refs., 5 tabs.

  20. Compound dual radiation action theory for 252Cf brachytherapy.

    PubMed

    Wang, C K; Zhang, X

    2004-01-01

    The existing dosimetry protocol that uses the concept of RBE for 252Cf brachytherapy contains large uncertainties. A new formula has been developed to correlate the biological effect (i.e. cell survival fraction) resulting from a mixed n + gamma radiation field with two physical quantities and two biological quantities. The formula is based on a pathway model evolved from that of the compound-dual-radiation-action (CDRA) theory, previously proposed by Rossi and Zaider. The new model employs the recently published data on radiation-induced DNA lesions. The new formula is capable of predicting quantitatively the synergistic effect caused by the interactions between neutron events and gamma ray events, and it is intended to be included into a new dosimetry protocol for future 252Cf brachytherapy.

  1. A pneumatic transfer system for special form {sup 252}Cf

    SciTech Connect

    Gehrke, R.J.; Berry, S.M.; Grafwallner, E.G.; Hoggan, J.M.

    1996-09-01

    A pneumatic transfer system has been developed for use with series 100 Special Form {sup 252}Cf. It was developed to reduce the exposure to personnel handling sources of {sup 252}Cf with masses up to 150 {micro}g by permitting remotely activated two-way transfer between the storage container and the irradiation position. The pneumatic transfer system also permits transfers for reproducible repetitive irradiation periods. In addition to the storage container equipped with quick-release fittings, the transfer system consists of an irradiation station, a control box with momentary contact switches to activate the air-pressure control valves and indicators to identify the location of the source, and connecting air hose and electrical wire. A source of 20 psig air and 110 volt electrical power are required for operation of the transfer system which can be easily moved and set up by one individual in 5 to 10 minutes. Tests have shown that rarely does a source become lodged in the transfer tubing, but two methods have been developed to handle incomplete transfers of the {sup 252}Cf source. The first method consists of closing one air vent to allow a pressure impulse to propel the source to the opposite side. The second method applies to those {sup 252}Cf capsules with a threaded or tapped end to which a small ferromagnetic piece can be attached; an incompletely transferred source in the transfer tube can then be guided to a position of safety by surrounding the transfer tubing containing the capsule with a horseshoe magnet attached to the end of a long pole.

  2. Orientation of fission fragments and anisotropy of {gamma}-Quanta emission

    SciTech Connect

    Barabanov, A.L.

    1994-07-01

    Experimental data on angular distributions of {gamma}-quanta emitted by fragments of binary and ternary spontaneous fission of {sup 252}Cf are analyzed. Their difference indicates that the fragment alignment is higher in ternary fission than that in binary fission. Consequences of a possible relation between the ternary fission mechanism and the excitation of collective modes at the stage of descent from the barrier to the scission point are discussed. 19 refs., 5 figs.

  3. TYPE A PACKAGE LIMITS OF SPONTANEOUS FISSION RADIONUCLIDES

    SciTech Connect

    Rawl, R.R.

    2001-09-17

    The maxima value of the depth dose coefficient for fission neutrons in ICRP Publication 21 was a reasonable estimator of the effective dose coefficient recently tabulated in ICRP Publication 74. Thus the inflation of the coefficient in the 1996 Q-System analysis (IAEA 2000b) for the purpose of being consistent with respect to ICRP guidance on the neutron weighting factor was unnecessary from the standpoint of the effective dose. The consequence resulted in an unnecessarily restrictive value of A{sub 1} for {sup 248}Cm, {sup 252}Cf, and {sup 254}Cf. The calculations presented here support a relaxation of the A{sub 1} limits for these radionuclides.

  4. Interstitial /sup 252/Cf neutron therapy for glioblastoma multiforme

    SciTech Connect

    Maruyama, Y.; Chin, H.W.; Young, A.B.; Bean, J.; Tibbs, P.; Beach, J.L.

    1982-12-01

    /sup 252/Cf brachytherapy has been combined with whole brain photon beam therapy to 6000 rads in 5-7 weeks. In early phase I studies, all patients selected for study tolerated the procedure and the subsequent photon beam therapy. All showed improvement in performance status and decreased tumor size by CT scan evaluation, but it became clear that these tumors are of large size and bulk, produce marked adjacent brain edema, and require individualized implant therapy as well as high-dose external beam irradiation if response is to occur.

  5. The collinear cluster tri-partition (CCT) of 252Cf (sf): New aspects from neutron gated data

    NASA Astrophysics Data System (ADS)

    Pyatkov, Yu. V.; Kamanin, D. V.; von Oertzen, W.; Alexandrov, A. A.; Alexandrova, I. A.; Falomkina, O. V.; Jacobs, N.; Kondratjev, N. A.; Kuznetsova, E. A.; Lavrova, Yu. E.; Malaza, V.; Ryabov, Yu. V.; Strekalovsky, O. V.; Tyukavkin, A. N.; Zhuchko, V. E.

    2012-07-01

    Results of two different experiments for the study of fission of 252Cf (sf) events in coincidence with neutrons are reported. Two time-of-flight-energy (TOF- E detectors systems have been used. The fission fragment masses were obtained in a double arm coincidence set-up, where the missing mass in the binary decay is used to characterise ternary fission as a collinear cluster tri-partition (CCT). The 3He filled neutron counters have been arranged so as to detect principally neutrons emitted from an isotropic source in the laboratory frame. The fission events connected to the larger experimental neutron multiplicities show a wide range in the missing-mass spectrum, down to α -particles, carbon and oxygen isotopes. These are linked with magic nuclei in the binary mass-mass correlations of the fission fragments. These neutron gated data are virtually free from background events from scattered binary fission fragments. The ungated spectra are compared to those of the previous data from our previous article (Eur. Phys. J. A. 45, 29 (2010)), the observed structures agree well with the manifestations of the collinear cluster tri-partition of 252Cf (sf) observed earlier. Several new families of the CCT modes are observed.

  6. Prompt Fission Gamma-ray Studies at DANCE

    NASA Astrophysics Data System (ADS)

    Jandel, M.; Rusev, G.; Bond, E. M.; Bredeweg, T. A.; Chadwick, M. B.; Couture, A.; Fowler, M. M.; Haight, R. C.; Kawano, T.; Keksis, A. L.; Mosby, S. M.; O'Donnell, J. M.; Rundberg, R. S.; Stetcu, I.; Talou, P.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Stoyer, M. A.; Haslett, R. J.; Henderson, R. A.; Becker, J. A.; Wu, C. Y.

    Measurements of correlated data on prompt-fission γ-rays (PFG) have been carried out for various actinide isotopes in recent years using the Detector for Advanced Neutron Capture Experiments (DANCE) at Los Alamos National Laboratory (LANL). We have developed a model that conveniently parametrizes the correlated data of γ-ray multiplicity and energy. New results on two- dimensional prompt-fission γ-ray multiplicity versus energy distributions from spontaneous fission on 252Cf and neutron-induced fission on 242mAm are presented together with previously obtained results on 233,235U and 239Pu. Correlated PFG data from 252Cf are also compared to results of the detailed theoretical model developed at LANL, for different thresholds of PFG energies. Future plans to measure correlated data on fission fragments, prompt fission neutrons and γ-rays at DANCE are presented.

  7. Potential Energy Calculations for Collinear Cluster Tripartition Fission Events

    NASA Astrophysics Data System (ADS)

    Unzhakova, A. V.; Pashkevich, V. V.; Pyatkov, Y. V.

    2014-09-01

    Strutinsky shell correction calculations were performed to describe the recent experimental results on collinear ternary fission. Collinear Cluster Tripartion fission events were studied experimentally in neutron induced fission of 235U, where the missing mass in the detected binary decay was suggested to characterize fission event as a collinear tripartition; and in spontaneous fission of 252Cf, where the direct detection of the three fission fragments has been used to confirm the existence of the Collinear Cluster Tripartition channel with a probability of 4.7×10-3 relative to the binary fission events.

  8. Moderated 252Cf neutron energy spectra in brain tissue and calculated boron neutron capture dose.

    PubMed

    Rivard, Mark J; Zamenhof, Robert G

    2004-11-01

    While there is significant clinical experience using both low- and high-dose (252)Cf brachytherapy, combination therapy using (10)B for neutron capture therapy-enhanced (252)Cf brachytherapy has not been performed. Monte Carlo calculations were performed in a brain phantom (ICRU 44 brain tissue) to evaluate the dose enhancement predicted for a range of (10)B concentrations over a range of distances from a clinical (252)Cf source. These results were compared to experimental measurements and calculations published in the literature. For (10)B concentrations 252)Cf fast neutron dose.

  9. Basic results of investigations of scission neutrons in nuclear fission at low excitation energies

    SciTech Connect

    Petrov, G. A. Gagarski, A. M.; Guseva, I. S.; Sokolov, V. E.; Val'ski, G. V.; Vorobiev, A. S.; Krinitcin, D. O.; Shcherbakov, O. A.; Nikolaev, D. V.; Pleva, Yu. S.; Petrova, V. I.; Zavarukhina, T. A.

    2008-07-15

    To estimate the main characteristics of neutrons emitted shortly before the scission of a fissioning nucleus, various experiments sensitive to the presence of these scission neutrons in thermal-neutron-induced fission of {sup 235}U and spontaneous fission of {sup 252}Cf were performed. The results of the experiments were analyzed within theoretical calculations allowing for various possible neutron-emission mechanisms, including the possibility of the emergence of neutrons from the scission of a nucleus.

  10. Spontaneous fission properties and lifetime systematics

    SciTech Connect

    Hoffman, D.C.

    1989-03-01

    Half-lives for spontaneous fission of nuclides with even and odd numbers of particles are compared with recent theoretical calculations. A summary of odd particle hindrance factors is given. The most recent measurements of kinetic-energy and mass distributions and neutron emission for spontaneous fission of the heaviest nuclides are summarized and discussed. 51 refs., 9 figs.

  11. Measurement of the 250Cf component in a 252Cf neutron source at KRISS.

    PubMed

    Kim, Jungho; Park, Hyeonseo; Choi, Kil-Oung

    2014-10-01

    Neutron emission rate measurements have been carried out at the Korea Research Institute of Standards and Science using a manganese sulphate bath system for (252)Cf and (241)Am-Be sources since 2004. The relative measurement method was chosen in 2012, and the neutron emission rates agreed with those by the absolute measurement method within uncertainties. The neutron emission rate of an old (252)Cf source has been measured three times: in 2004, 2009 and 2012. The (250)Cf component was fitted to a double-exponential function of (252)Cf+(250)Cf, and the ratio of the (250)Cf component to the (252)Cf component was estimated to be 7.8 % in 2004 and 46.8 % in 2012. Underestimation of the neutron emission rates of old (252)Cf sources can be corrected if the neutron emission rate of the (250)Cf component is taken into account.

  12. A radiobiological model for the relative biological effectiveness of high-dose-rate 252Cf brachytherapy.

    PubMed

    Rivard, Mark J; Melhus, Christopher S; Zinkin, Heather D; Stapleford, Liza J; Evans, Krista E; Wazer, David E; Odlozilíková, Anna

    2005-09-01

    While there is significant clinical experience using both low- and high-dose-rate 252Cf brachytherapy, there are minimal data regarding values for the neutron relative biological effectiveness (RBE) with both modalities. The aim of this research was to derive a radiobiological model for 252Cf neutron RBE and to compare these results with neutron RBE values used clinically in Russia. The linear-quadratic (LQ) model was used as the basis to characterize cell survival after irradiation, with identical cell killing rates (S(N) = S(gamma)) between 252Cf neutrons and photons used for derivation of RBE. Using this equality, a relationship among neutron dose and LQ radiobiological parameter (i.e., alpha(N), beta(N), alpha(gamma), beta(gamma)) was obtained without the need to specify the photon dose. These results were used to derive the 252Cf neutron RBE, which was then compared with Russian neutron RBE values. The 252Cf neutron RBE was determined after incorporating the LQ radiobiological parameters obtained from cell survival studies with fast neutrons and teletherapy photons. For single-fraction high-dose-rate neutron doses of 0.5, 1.0, 1.5 and 2.0 Gy, the total biologically equivalent doses were 1.8, 3.4, 4.7 and 6.0 RBE Gy with 252Cf neutron RBE values of 3.2, 2.9, 2.7 and 2.5, respectively. Using clinical data for late-responding reactions from 252Cf, Russian investigators created an empirical model that predicted high-dose-rate 252Cf neutron RBE values ranging from 3.6 to 2.9 for similar doses and fractionation schemes and observed that 252Cf neutron RBE increases with the number of treatment fractions. Using these relationships, our results were in general concordance with high-dose-rate 252Cf RBE values obtained from Russian clinical experience.

  13. Replacing a 252Cf source with a neutron generator in a shuffler - a conceptual design performed with MCNPX

    SciTech Connect

    Schear, Melissa A; Tobin, Stephen J

    2009-01-01

    The {sup 252}Cf shuffler has been widely used in nuclear safeguards and radioactive waste management to assay fissile isotopes, such as {sup 235}U or {sup 239}Pu, present in a variety of samples, ranging from small cans of uranium waste to metal samples weighing several kilograms. Like other non-destructive assay instruments, the shuffler uses an interrogating neutron source to induce fissions in the sample. Although shufflers with {sup 252}Cf sources have been reliably used for several decades, replacing this isotopic source with a neutron generator presents some distinct advantages. Neutron generators can be run in a continuous or pulsed mode, and may be turned off, eliminating the need for shielding and a shuffling mechanism in the shuffler. There is also essentially no dose to personnel during installation, and no reliance on the availability of {sup 252}Cf. Despite these advantages, the more energetic neutrons emitted from the neutron generator (141 MeV for D-T generators) present some challenges for certain material types. For example when the enrichment of a uranium sample is unknown, the fission of {sup 238}U is generally undesirable. Since measuring uranium is one of the main uses of a shuffler, reducing the delayed neutron contribution from {sup 238}U is desirable. Hence, the shuffler hardware must be modified to accommodate a moderator configuration near the source to tailor the interrogating spectrum in a manner which promotes sub-threshold fissions (below 1 MeV) but avoids the over-moderation of the interrogating neutrons so as to avoid self-shielding. In this study, where there are many material and geometry combinations, the Monte Carlo N-Particle eXtended (MCNPX) transport code was used to model, design, and optimize the moderator configuration within the shuffler geometry. The code is then used to evaluate and compare the assay performances of both the modified shuffler and the current {sup 252}Cf shuffler designs for different test samples. The

  14. All possible ternary fragmentations of {sup 252}Cf in collinear configuration

    SciTech Connect

    Manimaran, K.; Balasubramaniam, M.

    2011-03-15

    All possible ternary fragmentations in fission of {sup 252}Cf are studied in collinear configuration within a spherical approximation using the recently proposed ''three cluster model.'' The potential energy surface of collinear configuration exhibits a strong valley around {sup 48}Ca and its neighboring nuclei {sup 50}Ca, {sup 54}Ti, and {sup 60}Cr. Such strong minima are not seen in the potential energy surface of an equatorial configuration. As a consequence of strong minima in the potential, the overall relative yield is higher for the ternary fragmentation with {sup 48}Ca, {sup 50}Ca, {sup 54}Ti, {sup 60}Cr, and {sup 82}Ge as the third fragment. The results of potential energy and relative yield calculations reveal that collinear configuration increases the probability of emission of heavy fragments like {sup 48}Ca (doubly magic nucleus) and its neighboring nuclei as the third fragment. The obtained results indicate that the collinear configuration is the preferred configuration for intermediate nuclei ({sup 48}Ca, {sup 50}Ca, {sup 54}Ti, and {sup 60}Cr) as the third fragment in particle accompanied fission while the equatorial configuration may be a preferred configuration for light nuclei ({sup 4}He, {sup 10}Be) as the third fragment.

  15. /sup 252/Cf-source-driven neutron noise analysis method

    SciTech Connect

    Mihalczo, J.T.; King, W.T.; Blakeman, E.D.

    1985-01-01

    The /sup 252/Cf-source-driven neutron noise analysis method has been tested in a wide variety of experiments that have indicated the broad range of applicability of the method. The neutron multiplication factor k/sub eff/ has been satisfactorily detemined for a variety of materials including uranium metal, light water reactor fuel pins, fissile solutions, fuel plates in water, and interacting cylinders. For a uranyl nitrate solution tank which is typical of a fuel processing or reprocessing plant, the k/sub eff/ values were satisfactorily determined for values between 0.92 and 0.5 using a simple point kinetics interpretation of the experimental data. The short measurement times, in several cases as low as 1 min, have shown that the development of this method can lead to a practical subcriticality monitor for many in-plant applications. The further development of the method will require experiments oriented toward particular applications including dynamic experiments and the development of theoretical methods to predict the experimental observables.

  16. Spontaneous fission of 256Rf, new data

    NASA Astrophysics Data System (ADS)

    Svirikhin, A. I.; Yeremin, A. V.; Izosimov, I. N.; Isaev, A. V.; Kuznetsov, A. N.; Malyshev, O. N.; Popeko, A. G.; Popov, Yu. A.; Sokol, E. A.; Chelnokov, M. L.; Chepigin, V. I.; Andel, B.; Asfari, M. Z.; Gall, B.; Yoshihiro, N.; Kalaninova, Z.; Mullins, S.; Piot, J.; Stefanova, E.; Tonev, D.

    2016-07-01

    Spontaneous fission properties of the short-lived neutron-deficient 256Rf nucleus produced in the complete fusion reaction with a beam of multiply charged heavy 50Ti ions from the U-400 cyclotron (FLNR, JINR) are experimentally investigated. Its half-life and decay branching ratio are measured. The average number of neutrons per spontaneous fission of 256Rf (bar v = 4.47 ± 0.09) is determined for the first time.

  17. A multiple parallel-plate avalanche counter for fission-fragment detection

    NASA Astrophysics Data System (ADS)

    Wu, C. Y.; Henderson, R. A.; Haight, R. C.; Lee, H. Y.; Taddeucci, T. N.; Bucher, B.; Chyzh, A.; Devlin, M.; Fotiades, N.; Kwan, E.; O'Donnell, J. M.; Perdue, B. A.; Ullmann, J. L.

    2015-09-01

    A new low-mass multiple gas-filled parallel-plate avalanche counter for the fission-fragment detection has been developed to mark the fission occurrence in measurements of the prompt fission neutron energy spectrum as a function of incident neutron energy. It was used successfully for the neutron-induced fission of 235U and 239Pu with a total mass near 100 mg each and the spontaneous fission of 252Cf. Both the incident neutron energy and the prompt fission neutron energy are measured by using the time-of-flight method. The design and performance of this avalanche counter are described.

  18. Fission Measurements with Dance

    NASA Astrophysics Data System (ADS)

    Jandel, M.; Bredeweg, T. A.; Fowler, M. M.; Bond, E. M.; Chadwick, M. B.; Clement, R. R.; Couture, A.; O'Donnell, J. M.; Haight, R. C.; Keksis, A. L.; Reifarth, R.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Wouters, J. M.; Agvaanluvsan, U.; Dashdorj, D.; Macri, R. A.; Parker, W. E.; Wilk, P. A.; Wu, C. Y.; Becker, J. A.; Angell, C. T.; Tonchev, A. P.; Baker, J. D.

    2008-08-01

    Neutron capture cross section measurements on actinides are complicated by the presence of neutron-induced fission. An efficient fission tagging detector used in coincidence with the Detector for Advanced Neutron Capture Experiments (DANCE) provides a powerful tool in undertaking simultaneous measurements of (n,γ) and (n,f) cross sections. Preliminary results on 235U(n,γ) and (n,f) and 242mAm(n,f) cross sections measured with DANCE and a custom fission-tagging parallel plate avalanche counter (PPAC) are presented. Additional measurements of γ-ray cluster multiplicity distributions for neutron-induced fission of 235U and 242mAm and spontaneous fission of 252Cf are shown, as well as γ-ray energy and average γ-ray energy distributions.

  19. A comparison of the expected costs of high dose rate brachytherapy using 252Cf versus 192Ir.

    PubMed

    Rivard, Mark J; Kirk, Bernadette L; Stapleford, Liza J; Wazer, David E

    2004-12-01

    A cost analysis to compare high dose rate (HDR) brachytherapy using either californium-252 (252Cf) or 192Ir was performed to determine the prospects of widespread clinical implementation of HDR 252Cf. Interest in the neutron-emitting 252Cf radioisotope as a radiotherapy nuclide has undergone a resurgence given recent efforts to fabricate HDR remotely afterloaded sources, and other efforts to create a miniature source for improved accessibility to a variety of anatomic sites. Therefore, HDR 252Cf brachytherapy may prove to be a potential rival to the use of HDR 192Ir remotely afterloaded brachytherapy--the current standard-of-care treatment modality using HDR brachytherapy. Considering the possible improvements in clinical efficacy using HDR 252Cf brachytherapy and the enormous costs of other high-LET radiation sources, the cost differences between 252Cf and 192Ir may be well-justified.

  20. Description of the /sup 252/Cf(sf) neutron spectrum in the framework of a generalized Madland-Nix model

    SciTech Connect

    Marten, H.; Seeliger, D.

    1986-08-01

    The Madland-Nix model (MNM) for the calculation of fission neutron spectra is modified considering the dependence on fragment mass number A. Further, an approximation of this generalized Madland-Nix model (GMNM) that takes into account the different center-of-mass system spectra for the light and heavy fragment groups is discussed. These new calculations are compared with two versions of the original MNM. In particular, the level density parameter, which was adjusted by fitting the calculated spectra to a Maxwellian distribution deduced from experimental data, becomes more reasonable in the framework of the GMNM. The results of the different model calculations are compared with experimental data on the /sup 252/Cf(sf) neutron spectrum in the 0.1- to 20-MeV energy range.

  1. AN INTERLABORATORY COMPARISON ON THE DETERMINATION OF 241Am, 244Cm AND 252Cf IN URINE.

    PubMed

    Gerstmann, Udo C; Taubner, Kerstin; Hartmann, Martina

    2016-09-01

    An intercomparison exercise on the determination of (241)Am, (244)Cm and (252)Cf in urine was performed. Since it was designed with regard to emergency preparedness, the detection limit for each nuclide was set to 0.1 Bq per 24-h urine sample. Most of the participating laboratories were established bioassay laboratories. However, some laboratories that routinely determine (241)Am only in environmental samples were also invited in order to explore their potential for emergency bioassay analysis. Another aspect of the intercomparison was to investigate the performance of all laboratories concerning the chemical yields of the (243)Am tracer in comparison with (244)Cm and (252)Cf. In summary, both types of laboratories showed good results. There was a negative bias for the results of (244)Cm and (252)Cf, which can be explained by slightly different radiochemical behaviours of americium, curium and californium and which is in agreement with results reported in the literature. PMID:26535001

  2. Fluence-to-dose equivalent conversion factors for polyethylene-moderated {sup 252}Cf

    SciTech Connect

    Tanner, J.E.; Soldat, K.L.; Stewart, R.D.; Casson, W.H.

    1994-04-01

    Neutron measurements and calculations were conducted to characterize the polyethylene-moderated {sup 252}Cf source at Oak Ridge National Laboratory`s Radiation Calibration Laboratory (RADCAL). The 12-inch-diameter polyethylene sphere produces a highly scattered neutron spectrum which is more representative of most radiation fields found in the workplace than the D{sub 2}O-moderated {sup 252}Cf neutron spectrum typically used for dosimeter calibration. However, the energy-dependent fluence and dose equivalent must be well known before using such a source for radiation protection purposes. The measurements and calculations were performed as independent checks of the desired quantities which were the flux, the absorbed dose rate, the dose equivalent rate, and the average energy. These quantities were determined for the polyethylene sphere with and without an outer cadmium shell and compared with a D{sub 2}O-moderated {sup 252}Cf source.

  3. Spontaneous fission of /sup 259/Fm

    SciTech Connect

    Hulet, E.K.; Lougheed, R.W.; Landrum, J.H.; Wild, J.F.; Hoffman, D.C.; Weber, J.; Wilhelmy, J.B.

    1980-03-01

    A 1.5-s spontaneous fission activity has been produced by irradiating /sup 257/Fm with 16-MeV tritons. On the basis of formation cross sections, fission half-life systematics, and the identification of other possible products, this 1.5-s activity has been attributed to /sup 259/Fm formed by the reaction /sup 257/Fm(t,p)/sup 259/Fm. /sup 259/Fm is the heaviest known isotope of Fm and has more neutrons than any other nuclide thus far identified. This measurement of the spontaneous fission of /sup 259/Fm is the first to show a narrow, predominantly symmetric, mass division from spontaneous fission. It is accompanied by a very high kinetic energy, the most probable total kinetic energy being 242 +- 6 MeV. These features show a marked acceleration in the trend toward more symmetric mass division and higher total kinetic energies than have been observed previously for the Fm isotopes as the mass increased.

  4. Design of a setup for 252Cf neutron source for storage and analysis purpose

    NASA Astrophysics Data System (ADS)

    Hei, Daqian; Zhuang, Haocheng; Jia, Wenbao; Cheng, Can; Jiang, Zhou; Wang, Hongtao; Chen, Da

    2016-11-01

    252Cf is a reliable isotopic neutron source and widely used in the prompt gamma ray neutron activation analysis (PGNAA) technique. A cylindrical barrel made by polymethyl methacrylate contained with the boric acid solution was designed for storage and application of a 5 μg 252Cf neutron source. The size of the setup was optimized with Monte Carlo code. The experiments were performed and the results showed the doses were reduced with the setup and less than the allowable limit. The intensity and collimating radius of the neutron beam could also be adjusted through different collimator.

  5. Water-extended polyester neutron shield for a 252Cf neutron source.

    PubMed

    Vega-Carrillo, H R; Manzanares-Acuña, E; Hernández-Dávila, V M; Gallego, E; Lorente, A; Donaire, I

    2007-01-01

    A Monte Carlo study to determine the shielding features to neutrons of water-extended polyester was carried out. During calculations, (252)Cf and shielding were modelled and the neutron spectra as well as the H(10) were calculated in four sites. The calculation was extended to include a water shielding, the source in vacuum and in air. Besides neutron shielding characteristics, the Kerma in air due to gammas emitted by (252)Cf and due to capture gamma rays in the shielding were included.

  6. A Fission Time Projection Chamber for High Precision Cross Section Measurements

    NASA Astrophysics Data System (ADS)

    Snyder, Lucas; Greife, Uwe

    2010-11-01

    The design of next generation nuclear reactors and other nuclear applications are increasingly dependent on advanced simulations. Sensitivity studies have shown a need for high precision nuclear data to improve the predictive capabilities of these simulations. The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has constructed and is currently testing a prototype Time Projection Chamber (TPC) designed to measure fission cross sections to a higher accuracy than is capable with existing technology. In this talk, I will discuss the status of the fission TPC and progress on collecting the first set of data from ^252Cf spontaneous fission.

  7. Spontaneous fission properties of the heavy elements: Bimodal fission

    SciTech Connect

    Hulet, E.K.

    1988-11-11

    We have measured the mass and kinetic-energy distributions from the spontaneous fission of SVYFm, SVYNo, SVZMd, SWMd, SW(104), and SWSNo. All are observed to fission with a symmetrical division of mass, whereas the total-kinetic-energy (TKE) distributions strongly deviated from the Gaussian shape characteristically found in the fission of all other actinides. When the TKE distributions are resolved into two Gaussian's, the constituent peaks lie near 200 and near 233 MeV. We conclude two modes or bimodal fission is occurring in five of the six nuclides studied. Both modes are possible in the same nuclide, but one generally predominates. We also conclude the low-energy but mass-symmetrical mode is likely to extend to far heavier nuclei; while the high-energy mode will be restricted to a smaller region, a region of nuclei defined by the proximity of the fragments to the strong neutron and proton shells in TSSn. 21 refs., 7 figs., 1 tab.

  8. Comparative toxicity of /sup 226/Ra, /sup 239/Pu, /sup 241/Am, /sup 249/Cf, and /sup 252/Cf in C57BL/Do black and albino mice

    SciTech Connect

    Taylor, G.N.; Mays, C.W.; Lloyd, R.D.; Gardner, P.A.; TAlbot, L.R.; McFarland, S.S.; Pollard, T.A.; Atherton, D.R.; vanMoorhem, D.; Brammer, D.

    1983-09-01

    Groups of C57BL/Do (black and albino) mice were injected with graded activities of /sup 226/Ra, /sup 239/Pu, /sup 241/Am, /sup 249/Cf, or /sup 252/Cf and were followed throughout life. Bone sarcoma was the principal radiation-induced end point, and the risks associated with average skeletal doses of the four transuranium radionuclides, relative to radium, were determined. The relative biological effectiveness (RBE) was calculated for each emitter by dividing its risk coefficient (bone sarcomas per 10/sup 6/ mouse-rad) by the risk coefficient for /sup 226/Ra. Combined data for males and females in both black and albino mice gave the following values +- SD for the RBE relative to /sup 226/Ra = 1.0: /sup 239/Pu = 15.3 +- 3.9, /sup 241/Am = 4.9 +- 1.4, /sup 249/Cf = 5.0 +- 1.4, and /sup 252/Cf = 2.6 +- 0.8. About 70% of the tumors occurred in the axial skeleton, and the risk coefficient for females averaged about four times higher than for males when all five nuclides were included. The RBE of fission fragment irradiation from /sup 252/Cf for cancer induction, relative to ..cap alpha.. irradiation, for the combined data in all of the animals given /sup 252/Cf and /sup 249/Cf, was 0.02 +- 0.28, in agreement with the calculated theoretical value of 0.03, based on the ratio of summed track lengths in tissue.

  9. Comparative toxicity of /sup 226/Ra, /sup 239/Pu, /sup 241/Am, /sup 249/Cf, and /sup 252/Cf in C57BL/Do black and albino mice

    SciTech Connect

    Taylor, G.N.; Mays, C.W.; Lloyd, R.D.; Gardner, P.A.; Talbot, L.R.; McFarland, S.S.; Pollard, I.A.; Atherton, D.R.; VanMoorhem, D.; Brammer, D.

    1983-09-01

    Groups of C57BL/Do (black and albino) mice were injected with graded activities of /sup 226/Ra, /sup 239/Pu, /sup 241/Am, /sup 249/Cf, or /sup 252/Cf and were followed throughout life. Bone sarcoma was the principal radiation-induced end point, and the risks associated with average skeletal doses of the four transuranium radionuclides, relative to radium, were determined. The relative biological effectiveness (RBE) was calculated for each emitter by dividing its risk coefficient (bone sarcomas per 10(/sup 6/) mouse-rad) by the risk coefficient for /sup 226/Ra. Combined data for males and females in both black and albino mice gave the following values +/- SD for the RBE relative to /sup 226/Ra . 1.0: /sup 239/Pu . 15.3 +/- 3.9, /sup 241/Am . 4.9 +/- 1.4, /sup 249/Cf . 5.0 +/- 1.4, and /sup 252/Cf . 2.6 +/- 0.8. About 70% of the tumors occurred in the axial skeleton, and the risk coefficient for females averaged about four times higher than for males when all five nuclides were included. The RBE of fission fragment irradiation from /sup 252/Cf for cancer induction, relative to alpha irradiation, for the combined data in all of the animals given /sup 252/Cf and /sup 249/Cf, was 0.02 +/- 0.28, in agreement with the calculated theoretical value of 0.03, based on the ratio of summed track lengths in tissue.

  10. On the use of a (252Cf-3He) assembly for landmine detection by the neutron back-scattering method.

    PubMed

    Elsheikh, N; Viesti, G; ElAgib, I; Habbani, F

    2012-04-01

    Experiments were carried out to optimize the performance of the neutron back-scattering (NBS) technique in landmine detection using an assembly consisting of three different layers placed above a (252)Cf neuron source, producing about 10(4)s(-1), in conjunction with a (3)He detector. The assembly was optimized experimentally. The selected assembly configuration was then examined against different (252)Cf stand-off distances and mine burial depths using dummy landmines. Furthermore, Monte Carlo simulations were performed to study the effect of the shield when a (252)Cf source in the range 10(4)-10(7)s(-1) was employed, and to optimize the geometry for future prototypes.

  11. Brazilian gamma-neutron dosemeter: response to 241AmBe and 252Cf neutron sources.

    PubMed

    Souto, E B; Campos, L L

    2011-03-01

    With the aim of improving the monitoring of workers potentially exposed to neutron radiation in Brazil, the IPEN/CNEN-SP in association with PRO-RAD designed and developed a passive individual gamma-neutron mixed-field dosemeter calibrated to be used to (241)AmBe sources. To verify the dosimetry system response to different neutron spectra, prototypes were irradiated with a (252)Cf source and evaluated using the dose-calculation algorithm developed for (241)AmBe sources.

  12. Measured microdosimetric spectra and therapeutic potential of boron neutron capture enhancement of 252Cf brachytherapy.

    PubMed

    Burmeister, J; Kota, C; Maughan, R L

    2005-09-01

    Californium-252 is a neutron-emitting radioisotope used as a brachytherapy source for radioresistant tumors. Presented here are microdosimetric spectra measured as a function of simulated site diameter and distance from applicator tube 252Cf sources. These spectra were measured using miniature tissue-equivalent proportional counters (TEPCs). An investigation of the clinical potential of boron neutron capture (BNC) enhancement of 252Cf brachytherapy is also provided. The absorbed dose from the BNC reaction was measured using a boron-loaded miniature TEPC. Measured neutron, photon and BNC absorbed dose components are provided as a function of distance from the source. In general, the absorbed dose results show good agreement with results from other measurement techniques. A concomitant boost to 252Cf brachytherapy may be provided through the use of the BNC reaction. The potential magnitude of this BNC enhancement increases with increasing distance from the source and is capable of providing a therapeutic gain greater than 30% at a distance of 5 cm from the source, assuming currently achievable boron concentrations.

  13. Spontaneous fission half-lives and their systematics

    SciTech Connect

    Holden, N.E.

    1998-03-01

    Spontaneous fission is a phenomenon exhibited by heavy nuclei, which can be a major mode of decay of nuclei of elements heavier than thorium and can be a determining factor in their stability. For purposes of this paper, spontaneous fission will be considered a process in which a nucleus breaks up into two approximately equal parts. The emission of light nuclei or heavy ions such as {sup 12}C, {sup 16}O, or {sup 32}S will not be considered. This radioactive decay mode is often much smaller than the spontaneous fission decay mode, although this is not true in all cases. Barwick noted that this might indicate that the assumed half-life for spontaneous fission of some older experiments might be partially due to heavy fragment radioactivity. Other than taking note of this potential correction to spontaneous fission half-lives, this decay mode of heavy fragment radioactivity will be ignored. Excited states of some heavy nuclei may decay via spontaneous fission. These so-called fission isomers will not be discussed here. Electron capture (EC) or beta-delayed fission is a process in which prompt fission of a sufficiently excited daughter state occurs following population by EC or beta decay. The fission activity will appear to decay with the half-life of the parent and was earlier confused in some cases with SF. This process has been discussed in detail in a review and will not be considered in this paper.

  14. Neutron Multiplicity At Spontaneous Fission Of 246Fm

    NASA Astrophysics Data System (ADS)

    Svirikhin, A. I.; Yeremin, A. V.; Chelnokov, M. L.; Chepigin, V. I.; Izosimov, I. V.; Katrasev, D. E.; Malyshev, O. N.; Minkova, A.; Popeko, A. G.; Sokol, E. A.

    2010-04-01

    For experiments aimed at the study of spontaneous fission of transfermium nuclei improvements in the focal plane detector system of recoil separa tor VASSILISSA have been made. The neutron detector consisting of 54 3He -filled counters has been mounted around the focal plane detector chamber. The multiplicity of prompt neutrons emitted in spontaneous fission of 246 Fm was measured.

  15. A New Method of Prompt Fission Neutron Energy Spectrum Unfolding

    SciTech Connect

    Zeynalova, O. V.; Zeynalov, Sh.; Hambsch, F.-J.; Oberstedt, S.

    2010-11-25

    The prompt neutron emission in spontaneous fission of {sup 252}Cf has been investigated applying digital signal electronics along with associated digital signal processing algorithms. The goal was to find out the reasons of a long time existing discrepancy between theoretical calculations and the measurements of prompt fission neutron (PFN) emission dependence on the total kinetic energy (TKE) of fission fragments (FF). On the one hand the {sup 252}Cf(sf) reaction is one of the main references for nuclear data, on the other hand the understanding of PFN emission mechanism is very important for nuclear fission theory. Using a twin Frisch-grid ionization chamber for fission fragment (FF) detection and a NE213-equivalent neutron detector in total about 10{sup 7} fission fragment-neutron coincidences have been registered. Fission fragment kinetic energy, mass and angular distribution, neutron time-of-flight and pulse shape have been investigated using a 12 bit waveform digitizer. The signal waveforms have been analyzed using digital signal processing algorithms. For the first time the dependence of the number of emitted neutrons as a function of total kinetic energy (TKE) of the fragments is in very good agreement with theoretical calculations in the range of TKE from 140-220 MeV.

  16. A new facility for non-destructive assay using a 252Cf source.

    PubMed

    Stevanato, L; Caldogno, M; Dima, R; Fabris, D; Hao, Xin; Lunardon, M; Moretto, S; Nebbia, G; Pesente, S; Pino, F; Sajo-Bohus, L; Viesti, G

    2013-03-01

    A new laboratory facility for non-destructive analysis (NDA) using a time-tagged (252)Cf source is presented. The system is designed to analyze samples having maximum size of about 20 × 25 cm(2), the material recognition being obtained by measuring simultaneously total and energy dependent transmission of neutrons and gamma rays. The equipment technical characteristics and performances of the NDA system are presented, exploring also limits due to the sample thickness. Some recent applications in the field of cultural heritage are presented. PMID:23276691

  17. Test and evaluation results of the /sup 252/Cf shuffler at the Savannah River Plant

    SciTech Connect

    Crane, T.W.

    1981-03-01

    The /sup 252/Cf Shuffler, a nondestructive assay instrument employing californium neutron source irradiation and delayed-neutron counting, was developed for measuring /sup 235/U content of scrap and waste items generated at the Savannah River Plant (SRP) reactor fuel fabrication facility. The scrap and waste items include high-purity uranium-aluminum alloy ingots as well as pieces of castings, saw and lathe chips from machining operations, low-purity items such as oxides of uranium or uranium intermixed with flux materials found in recovery operations, and materials not recoverable at SRP such as floor sweepings or residues from the uranium scrap recovery operation. The uranium contains about 60% /sup 235/U with the remaining isotopes being /sup 236/U, /sup 238/U, and /sup 234/U in descending order. The test and evaluation at SRP concluded that the accuracy, safety, reliability, and ease of use made the /sup 252/Cf Shuffler a suitable instrument for routine use in an industrial, production-oriented plant.

  18. Brain tumour and infiltrations dosimetry of boron neutron capture therapy combined with 252Cf brachytherapy.

    PubMed

    Brandão, Sâmia F; Campos, Tarcísio P R

    2012-04-01

    This article presents a dosimetric investigation of boron neutron capture therapy (BNCT) combined with (252)Cf brachytherapy for brain tumour control. The study was conducted through computational simulation in MCNP5 code, using a precise and discrete voxel model of a human head, in which a hypothetical brain tumour was incorporated. A boron concentration ratio of 1:5 for healthy-tissue: tumour was considered. Absorbed and biologically weighted dose rates and neutron fluency in the voxel model were evaluated. The absorbed dose rate results were exported to SISCODES software, which generates the isodose surfaces on the brain. Analyses were performed to clarify the relevance of boron concentrations in occult infiltrations far from the target tumour, with boron concentration ratios of 1:1 up to 1:50 for healthy-tissue:infiltrations and healthy-tissue:tumour. The average biologically weighted dose rates at tumour area exceed up to 40 times the surrounding healthy tissue dose rates. In addition, the biologically weighted dose rates from boron have the main contribution at the infiltrations, especially far from primary tumour. In conclusion, BNCT combined with (252)Cf brachytherapy is an alternative technique for brain tumour treatment because it intensifies dose deposition at the tumour and at infiltrations, sparing healthy brain tissue.

  19. Applications of Event-by-Event Fission Modeling with FREYA

    SciTech Connect

    Vogt, R; Randrup, J

    2011-09-16

    The recently developed code FREYA (Fission Reaction Event Yield Algorithm) generates large samples of complete fission events, consisting of two receding product nuclei as well as a number of neutrons and photons, all with complete kinematic information. Thus it is possible to calculate arbitrary correlation observables whose behavior may provide unique insight into the fission process. We first discuss the present status of FREYA, which has now been extended to include spontaneous fission. Concentrating on {sup 239}Pu(n{sub th},f), {sup 240}Pu(sf) and {sup 252}Cf(sf), we discuss the neutron multiplicity correlations, the dependence of the neutron energy spectrum on the neutron multiplicity, and the relationship between the fragment kinetic energy and the number of neutrons and their energies. We also suggest novel fission observables that could be measured with modern detectors.

  20. Application of 252Cf plasma desorption mass spectrometry in dental research

    NASA Astrophysics Data System (ADS)

    Fritsch, Hans-Walter; Schmidt, Lothar; Köhl, Peter; Jungclas, Hartmut; Duschner, Heins

    1993-07-01

    Topically applied fluorides introduced in dental hygiene products elevate the concentration levels of fluoride in oral fluids and thus also affect chemical reactions of enamel de- and remineralisation. The chemical reactions on the surface of tooth enamel still are a subject of controversy. Here 252Cf-plasma desorption mass spectrometry and argon ion etching are used to analyse the molecular structure of the upper layes of enamel. The mass spectrum of untreated enamel is characterised by a series of cluster ions containing phosphate. It is evident that under certain conditions the molecular structure of the surface enamel is completely transformed by treatment with fluorides. The result of the degradation and precipitation processes is reflected by a total replacement of the phosphate by fluoride in the measured cluster ion distribution. Stepwise etching of the upper layers by Ar+ ions reveals the transition from a nearly pure CaF2 structure to the unchanged composition of the enamel mineral.

  1. Characteristics of the simulated workplace neutron fields using a 252Cf source surrounded with cylindrical moderators.

    PubMed

    Tsujimura, N; Yoshida, T

    2004-01-01

    The authors established the simulated workplace neutron fields using a 252Cf source surrounded with cylindrical moderators at the Japan Nuclear Cycle Development Institute (JNC), Tokai Works. The moderators are annular cylinders made of polymethyl methacrylate and steel. The neutron energy spectrum at the reference calibration point was evaluated from the calculations by MCNP-4B and the measurements by the Bonner multisphere spectrometer and the hydrogen-filled proportional counters. The calculated neutron spectra were in good agreements with the measured ones. These fields can provide the realistic neutron spectra similar to those encountered around the glove-boxes of the fabrication process of MOX (PuO2-UO2 mixed oxide) fuel.

  2. Neutron-induced fission: properties of prompt neutron and γ rays as a function of incident energy

    NASA Astrophysics Data System (ADS)

    Stetcu, I.; Talou, P.; Kawano, T.

    2016-06-01

    We have applied the Hauser-Feshbach statistical theory, in a Monte-Carlo implementation, to the de-excitation of fission fragments, obtaining a reasonable description of the characteristics of neutrons and gamma rays emitted before beta decays toward stability. Originally implemented for the spontaneous fission of 252Cf and the neutroninduced fission of 235U and 239Pu at thermal neutron energy, in this contribution we discuss the extension of the formalism to incident neutron energies up to 20 MeV. For the emission of pre-fission neutrons, at incident energies beyond second-chance fission, we take into account both the pre-equilibrium and statistical pre-fission components. Phenomenological parameterizations of mass, charge and TKE yields are used to obtain the initial conditions for the fission fragments that subsequently decay via neutron and emissions. We illustrate this approach for 239Pu(n,f).

  3. On the Effect of an Error in a Standard D2O-Moderated 252Cf Energy Spectrum

    SciTech Connect

    Frederick Cummings

    2009-12-01

    There appears to be an error in the neutron fluence for neutrons with energies between 9 and 10 MeV for the tabulated D2O-moderated 252Cf source in ISO 8529-1. The error contributes a total error to neutron dose values from this source of approximately 3%.

  4. A new facility for Non-Destructive Assay with a time-tagged {sup 252}Cf source

    SciTech Connect

    Stevanato, L.; Caldogno, M.; Hao Xin; Dima, R.; Fabris, D.; Nebbia, G.; Lunardon, M.; Moretto, S.; Pesente, S.; Viesti, G.; Sajo-Bohus, L.

    2010-08-04

    A new facility for non-destructive assay using a time-tagged {sup 252}Cf source is presented. The system is designed to analyze samples having maximum size of about 15x20 cm{sup 2}, the material recognition being obtained by measuring simultaneously transmission of neutrons and gamma rays.

  5. Pairing-induced speedup of nuclear spontaneous fission

    SciTech Connect

    Sadhukhan, Jhilam; Dobaczewski, J.; Nazarewicz, W.; Sheikh, J. A.; Baran, A.

    2014-12-22

    Collective inertia is strongly influenced at the level crossing at which the quantum system changes its microscopic configuration diabatically. Pairing correlations tend to make the large-amplitude nuclear collective motion more adiabatic by reducing the effect of these configuration changes. Competition between pairing and level crossing is thus expected to have a profound impact on spontaneous fission lifetimes. To elucidate the role of nucleonic pairing on spontaneous fission, we study the dynamic fission trajectories of 264Fm and 240Pu using the state-of-the-art self-consistent framework. We employ the superfluid nuclear density functional theory with the Skyrme energy density functional SkM* and a density-dependent pairing interaction. Along with shape variables, proton and neutron pairing correlations are taken as collective coordinates. The collective inertia tensor is calculated within the nonperturbative cranking approximation. The fission paths are obtained by using the least action principle in a four-dimensional collective space of shape and pairing coordinates. Pairing correlations are enhanced along the minimum-action fission path. For the symmetric fission of 264Fm, where the effect of triaxiality on the fission barrier is large, the geometry of the fission pathway in the space of the shape degrees of freedom is weakly impacted by pairing. This is not the case for 240Pu, where pairing fluctuations restore the axial symmetry of the dynamic fission trajectory. The minimum-action fission path is strongly impacted by nucleonic pairing. In some cases, the dynamical coupling between shape and pairing degrees of freedom can lead to a dramatic departure from the static picture. As a result, in the dynamical description of nuclear fission, particle-particle correlations should be considered on the same footing as those associated with shape degrees of freedom.

  6. Pairing-induced speedup of nuclear spontaneous fission

    DOE PAGES

    Sadhukhan, Jhilam; Dobaczewski, J.; Nazarewicz, W.; Sheikh, J. A.; Baran, A.

    2014-12-22

    Collective inertia is strongly influenced at the level crossing at which the quantum system changes its microscopic configuration diabatically. Pairing correlations tend to make the large-amplitude nuclear collective motion more adiabatic by reducing the effect of these configuration changes. Competition between pairing and level crossing is thus expected to have a profound impact on spontaneous fission lifetimes. To elucidate the role of nucleonic pairing on spontaneous fission, we study the dynamic fission trajectories of 264Fm and 240Pu using the state-of-the-art self-consistent framework. We employ the superfluid nuclear density functional theory with the Skyrme energy density functional SkM* and a density-dependentmore » pairing interaction. Along with shape variables, proton and neutron pairing correlations are taken as collective coordinates. The collective inertia tensor is calculated within the nonperturbative cranking approximation. The fission paths are obtained by using the least action principle in a four-dimensional collective space of shape and pairing coordinates. Pairing correlations are enhanced along the minimum-action fission path. For the symmetric fission of 264Fm, where the effect of triaxiality on the fission barrier is large, the geometry of the fission pathway in the space of the shape degrees of freedom is weakly impacted by pairing. This is not the case for 240Pu, where pairing fluctuations restore the axial symmetry of the dynamic fission trajectory. The minimum-action fission path is strongly impacted by nucleonic pairing. In some cases, the dynamical coupling between shape and pairing degrees of freedom can lead to a dramatic departure from the static picture. As a result, in the dynamical description of nuclear fission, particle-particle correlations should be considered on the same footing as those associated with shape degrees of freedom.« less

  7. The discovery and spontaneous fission properties of /sup 262/No

    SciTech Connect

    Lougheed, R.W.; Hulet, E.K.; Wild, J.F.; Moody, K.J.; Dougan, R.J.; Gannett, C.M.; Henderson, R.A.; Hoffman, D.C.; Lee, D.M.

    1989-04-19

    We have discovered /sup 262/No, as the electron capture daughter of /sup 262/Lr(t/sub 1/2/ = 216 m). This new isotope of nobelium decays by spontaneous fission with about a 5-ms half-life which is several orders of magnitude longer than recent theoretical estimates. We measured a sharply symmetric fission-fragment mass division and a bimodal total kinetic energy distribution; the high-energy symmetric-fission path was most abundant. /sup 262/No is the first nuclide with 160 neutrons to be discovered and is the closest to the N = 162 neutron subshell for which enhanced stability is predicted. 14 refs., 3 figs.

  8. Calibration of a Manganese Bath Relative to 252Cf Nu-Bar

    NASA Astrophysics Data System (ADS)

    Gilliam, David M.; Yue, Andrew T.; Scott Dewey, M.

    2009-08-01

    A large manganese sulfate bath is employed at the National Institute of Standards and Technology (NIST) to calibrate isotopic neutron sources relative to the national standard neutron source NBS-I. In the past few years many low-emission Cf-252 neutron sources have been calibrated for testing of neutron detectors for the U.S. Department of Homeland Security (DHS). The low-emission DHS sources are about a factor of 100 lower in emission rate than NBS-I, so that background fluctuations become more significant in making accurate calibrations. To verify and improve the calibrations relative to NBS-I, a new calibration for sealed Cf-252 neutron sources has been made by measuring the fission rate of a bare Cf-252 deposit and inferring its neutron emission rate from Cf-252 nu-bar, the well-established neutron multiplicity of spontaneous fission in Cf-252. The fission rate of the bare deposit was measured by counting fission fragments in vacuum with a surface barrier detector behind an aperture and spacer, which provided a well-defined solid angle for detection. A thin polyimide film was placed just above the Cf deposit to prevent contamination of the detector by self-sputtering of the Cf material in vacuum. Tests with additional layers of polyimide were performed to observe any perturbation in the detection efficiency due to scattering or absorption of alpha particles or fission fragments in the polyimide film. The increase in the background count rate due to accumulation of Cf on the polyimide film was less than 0.02% of the fission fragment count rate from the sample, at the end of all runs. It is estimated that this increase in background would have been about 150 times higher without the polyimide film. The sealed Cf source NIST-DHSA was compared to the bare source by relative neutron counting in an assembly of polyethylene moderator and He-3 detectors. The calibration via Cf-252 nu-bar gave a result that was 1.7% higher than the previous calibration relative to NBS

  9. Insights into nuclear structure and the fission process from spontaneous fission

    SciTech Connect

    Hamilton, J.H.; Butler-Moore, K.; Ramayya, A.V.

    1993-12-31

    The {gamma}-rays emitted following spontaneous and induced fission are rich sources of information about the structure of neutron-rich nuclei and about the fission process itself. The study of spontaneous fissioning isotopes with large Ge detector arrays are providing a wealth of such information as seen, for example, in recent reports. In this paper we present some of our most recent results on nuclear structure studies and conclusions on the fission process itself. In our work, we have employed in spontaneous fission, a triple gamma coincidence study for the first time and a high resolution, X-ray detector-{gamma}-coincidence study. These data provide powerful ways of separating the gamma rays which belong to a particular nucleus. The triple coincidence technique was used to uniquely identify the levels in {sup 136}Te and higher spin states in its N=84 isotones, {sup 138}Xe and {sup 140}Ba{sup 171}. Some other examples of the level structures observed in the low and high mass partners are presented, including a detailed analysis of the backbending of the moment of inertia in {sup 112,114,116}Pd. Finally, we present the first examples of how our analysis allows one to extract a detailed picture of the dependence of the angular momentum on the mass and atomic numbers of the fission fragments and of the long-sought neutron multiplicity distribution from zero-n to ten-n as a function of the charge and mass asymmetry.

  10. Fabrication of 50-mg /sup 252/Cf neutron sources for the FDA (Food and Drug Administration) activation analysis facility

    SciTech Connect

    Bigelow, J.E.; Cagle, E.B.; Knauer, J.B.

    1987-01-01

    The Transuranium Processing Plant (TPP) at ORNL has been requested by the Food and Drug Administration (FDA) to furnish 200 mg of /sup 252/Cf for use in their new activation analysis facility. This paper discusses the procedure to be employed in fabricating the californium into four neutron sources, each containing a nominal 50-mg of /sup 252/Cf. The ORNL Model LSD (Large, Stainless steel, Doubly encapsulated) neutron source consists of a 6.33-mm-diam aluminum pellet doubly encapsulated in Type 304L stainless steel. The pellet is comprised of an aluminum tube holding Cf/sub 2/O/sub 2/SO/sub 4/ microspheres confined by pressed aluminum powder. The microspheres are prepared in a separate vessel and then transferred into the specially designed aluminum tube prior to pressing.

  11. The sup 252 Cf(sf) neutron spectrum in the 5- to 20-MeV energy range

    SciTech Connect

    Marten, H.; Richter, D.; Seeliger, D. ); Fromm, W.D. ); Bottger, R.; Klein, H. )

    1990-11-01

    This paper reports on the {sup 252}Cf neutron spectrum measured at high energies with a miniature ionization chamber and two different NE-213 neutron detectors. The gamma-ray background and the main cosmic background caused by muons were suppressed by applying efficient pulse-shape discrimination. On the basis of two-dimensional spectroscopy of the neutron time-of-flight and scintillation pulse height, the sliding bias method is used to minimize experimental uncertainties. The experimental data, corrected for several systematic influences, confirm earlier results that show negative deviations from a reference Maxwellian distribution with a 1.42-MeV spectrum temperature for neutron energies above 6 MeV. Experimental results of this work are compared with various statistical model approaches to the {sup 252}Cf(sf) neutron spectrum.

  12. Evaluation of the characteristics of the neutron reference field using D2O-moderated 252Cf source.

    PubMed

    Kowatari, M; Fujii, K; Takahashi, M; Yoshizawa, M; Shimizu, S; Kawasaki, K; Yamaguchi, Y

    2007-01-01

    The ambient/personal dose equivalent per fluence for D(2)O moderated (252)Cf neutron source was determined by measurement. An appropriate subtraction of the scattered neutrons is required for the accurate measurement of direct neutrons. A cubic shadow object was used for the subtraction of the scattered neutrons from the surroundings. The scattered neutrons to be subtracted vary with the position of the shadow object due to the large volume of the source. Using the Monte Carlo code MCNP-4C, the optimum positions of the shadow object were surveyed for subtracting the scattered neutrons. The energy spectra of direct neutrons were measured in the optimum position. The dosimetric parameters for the D(2)O moderated (252)Cf neutron source were reasonable, taking into account the uncertainties of the parameters.

  13. Intracavitary moderator balloon combined with 252Cf brachytherapy and boron neutron capture therapy, improving dosimetry in brain tumour and infiltrations

    PubMed Central

    Brandão, S F

    2015-01-01

    Objective: This article proposes a combination of californium-252 (252Cf) brachytherapy, boron neutron capture therapy (BNCT) and an intracavitary moderator balloon catheter applied to brain tumour and infiltrations. Methods: Dosimetric evaluations were performed on three protocol set-ups: 252Cf brachytherapy combined with BNCT (Cf-BNCT); Cf-BNCT with a balloon catheter filled with light water (LWB) and the same set-up with heavy water (HWB). Results: Cf-BNCT-HWB has presented dosimetric advantages to Cf-BNCT-LWB and Cf-BNCT in infiltrations at 2.0–5.0 cm from the balloon surface. However, Cf-BNCT-LWB has shown superior dosimetry up to 2.0 cm from the balloon surface. Conclusion: Cf-BNCT-HWB and Cf-BNCT-LWB protocols provide a selective dose distribution for brain tumour and infiltrations, mainly further from the 252Cf source, sparing the normal brain tissue. Advances in knowledge: Malignant brain tumours grow rapidly and often spread to adjacent brain tissues, leading to death. Improvements in brain radiation protocols have been continuously achieved; however, brain tumour recurrence is observed in most cases. Cf-BNCT-LWB and Cf-BNCT-HWB represent new modalities for selectively combating brain tumour infiltrations and metastasis. PMID:25927876

  14. Neutron Capture and Fission Measurements on Actinides at DANCE

    NASA Astrophysics Data System (ADS)

    Chyzh, Andrii; Wu, Ching-Yen; Kwan, Elaine; Henderson, Rodger; Gostic, Julie; Ullmann, John; Jandel, Marian; Bredeweg, Todd; Couture, Aaron; Lee, Hye Young; Haight, Robert; O'Donnell, John

    2011-10-01

    Neutron capture and fission measurements on actinides are important in nuclear engineering and physics. DANCE (Detector for Advanced Neutron Capture Measurement build at LANL) together with PPAC (avalanche technique based fission tagging detector designed and fabricated at LLNL) were used to measure the prompt γ-ray energy and multiplicity distributions in the spontaneous fission of 252Cf. These measured spectra together with the unfolded ones will be presented. The unfolding technique will be described. In addition the 238Pu(n , γ) cross section will be presented, which was measured using DANCE alone and also is the first such measurement in a laboratory environment. This work was performed under the auspices of the US Department of Energy by Los Alamos National Laboratory under Contract DE-AC52-06NA25396 and Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

  15. Assay of Low-Enriched Uranium using Spontaneous Fission Neutrons

    SciTech Connect

    Zucker, M. S.; Fainberg, A.

    1980-01-01

    Low-enriched uranium oxide in bulk containers can be assayed for safeguards purposes, using the neutrons from spontaneous fission of 238U as a signature, to complement enrichment and mass measurement. The penetrability of the fast fission neutrons allows the inner portion of bulk samples to register. The measurement may also be useful for measuring moisture content, of significance in process control. The apparatus used can be the same as for neutron correlation counting for Pu assay. The neutron multiplication observed in 238U is of intrinsic interest.

  16. Coal liquefaction process streams characterization and evaluation: The application of {sup 252}Cf-plasma desorption mass spectrometry to analysis of direct coal liquefaction heavy products

    SciTech Connect

    Larsen, J.W.; Lapucha, A.R.

    1992-10-01

    This study demonstrated the feasibility of using {sup 252}Cf PDMS, GPC, and MPLC for the examination of the tetrahydrofuran (THF)-soluble portion of distillation resid materials derived from direct coal liquefaction. The {sup 252}Cf-PDMS technique was used to determine molecular weight distributions of twenty-five THF-soluble resids. In order to detemine if {sup 252}Cf-PDMS responds differently to different chemical classes of compounds, Lehigh separated five of the samples into chemically distinct fractions by MPLC, then analyzed the parent samples, their fractions, and the re-mixed fractions by {sup 252}Cf-PDMS and GPC. Irreversible alteration of the samples upon separation was noted by Lehigh. This was confirmed by use of gas chromatographic (GC) analyses. The noted irreversible alterations prevented a direct comparison of the remixed materials and the original samples. Thus, the selective response of {sup 252}Cf-PDMS to different chemical classes of compounds could not be confirmed or ruled out. The number average molecular weights (M{sub n}) obtained by {sup 252}Cf-PDMS and GPC agreed well. However, the weight average molecular weights (M{sub w}) obtained by GPC are always higher than the corresponding {sup 252}Cf-PDMS results. Number average molecular weights and weight average molecular weights obtained with {sup 252}Cf-PDMS and GPC were compared with those obtained by field ionization mass spectrometry (FIMS), previously reported by SRI International for the parent resid samples from which the Lehigh THF-soluble samples were derived.

  17. Coal liquefaction process streams characterization and evaluation: The application of [sup 252]Cf-plasma desorption mass spectrometry to analysis of direct coal liquefaction heavy products

    SciTech Connect

    Larsen, J.W.; Lapucha, A.R.

    1992-10-01

    This study demonstrated the feasibility of using [sup 252]Cf PDMS, GPC, and MPLC for the examination of the tetrahydrofuran (THF)-soluble portion of distillation resid materials derived from direct coal liquefaction. The [sup 252]Cf-PDMS technique was used to determine molecular weight distributions of twenty-five THF-soluble resids. In order to detemine if [sup 252]Cf-PDMS responds differently to different chemical classes of compounds, Lehigh separated five of the samples into chemically distinct fractions by MPLC, then analyzed the parent samples, their fractions, and the re-mixed fractions by [sup 252]Cf-PDMS and GPC. Irreversible alteration of the samples upon separation was noted by Lehigh. This was confirmed by use of gas chromatographic (GC) analyses. The noted irreversible alterations prevented a direct comparison of the remixed materials and the original samples. Thus, the selective response of [sup 252]Cf-PDMS to different chemical classes of compounds could not be confirmed or ruled out. The number average molecular weights (M[sub n]) obtained by [sup 252]Cf-PDMS and GPC agreed well. However, the weight average molecular weights (M[sub w]) obtained by GPC are always higher than the corresponding [sup 252]Cf-PDMS results. Number average molecular weights and weight average molecular weights obtained with [sup 252]Cf-PDMS and GPC were compared with those obtained by field ionization mass spectrometry (FIMS), previously reported by SRI International for the parent resid samples from which the Lehigh THF-soluble samples were derived.

  18. Spontaneous fission properties of 2. 9-s sup 256 No

    SciTech Connect

    Hoffman, D.C.; Lee, D.M.; Gregorich, K.E.; Nurmia, M.J.; Chadwick, R.B.; Chen, K.B.; Czerwinski, K.R.; Gannett, C.M.; Hall, H.L.; Henderson, R.A.; Kadkhodayan, B.; Kreek, S.A.; Leyba, J.D. Chemistry Department, University of California, Berkeley, Berkeley, California 94720)

    1990-02-01

    We have measured the mass and kinetic-energy distributions of fragments from the spontaneous fission of {sup 256}No produced via the {sup 248}Cm({sup 12}C,4{ital n}) reaction. The production cross section using 71-MeV {sup 12}C projectiles was found to be 250 nb. The total kinetic energy for spontaneous fission of {sup 256}No is 196{plus minus}3 MeV. The mass distribution is very broad (full width at half maximum of {similar to}50 mass units) with no appreciable decrease in yield for symmetric mass division. {sup 256}No seems to be the transition nucleus between the asymmetric mass division observed for spontaneous fission of the lighter No isotopes and the symmetric mass division observed for the heavier No isotopes. Its properties are similar to those of {sup 257}Fm, the isotope at which this transition occurs in the Fm isotopes, but the {sup 256}No mass distribution is broader than that for {sup 257}Fm, and its average total kinetic energy for symmetric mass division is about 15 MeV lower. We determined the half-life of {sup 256}No to be 2.91{plus minus}0.05 s by measuring its {alpha} decay. We measured a spontaneous fission to {alpha} ratio of 0.0053{sub {minus}0.0003}{sup +0.0006}, which gives a partial half-life for spontaneous fission of 550{sub {minus}70}{sup +40} s. An energy of 8.448{plus minus}0.006 MeV was measured for the {alpha}-particle decay to the ground state of {sup 252}Fm, allowing us to calculate the mass excess for {sup 256}No as 87820{plus minus}8 keV. The energy of the 2{sup +} rotational level in the {sup 252}Fm daughter is 47{plus minus}5 keV, and the intensity of the 8.402-MeV {alpha} group populating this level is (13{plus minus}2)%.

  19. New Results on Helium and Tritium Gas Production From Ternary Fission

    NASA Astrophysics Data System (ADS)

    Serot, O.; Wagemans, C.; Heyse, J.

    2005-05-01

    Ternary fission constitutes an important source of helium and tritium gas production in nuclear reactors and in used fuel elements. Data related to this production are therefore requested by nuclear industry. In the present paper, we report results from measurements of the 4He and 3H emission probabilities (denoted LRA/B and t/B, respectively). These measurements concern both thermal neutron-induced fission reactions as well as spontaneous fission decays. For spontaneous fission, data are reported for nuclides ranging from 238Pu up to 252Cf. For thermal neutron-induced fission, results cover target nuclei between 229Th and 251Cf. Based on these and other results, semi-empirical relations are proposed. These correlations are only valid if spontaneous fission data and neutron-induced fission data are considered separately, which shows the impact of the fissioning nucleus-excitation energy on the ternary particle-emission process. In this way, t/B and LRA/B values could be evaluated for fissioning systems not investigated so far. These results could be used for the ternary fission-yield evaluation of the JEFF3.1 library.

  20. Spontaneous fission of the superheavy nucleus 286Fl

    NASA Astrophysics Data System (ADS)

    Poenaru, D. N.; Gherghescu, R. A.

    2016-07-01

    The decimal logarithm of spontaneous fission half-life of the superheavy nucleus 286Fl experimentally determined is log10Tfexp(s ) =-0.632 . We present a method to calculate the half-life based on the cranking inertia and the deformation energy, functions of two independent surface coordinates, using the best asymmetric two center shell model. Spherical shapes are assumed. In the first stage we study the statics. At a given mass asymmetry up to about η =0.5 the potential barrier has a two hump shape, but for larger η it has only one hump. The touching point deformation energy versus mass asymmetry shows the three minima, produced by shell effects, corresponding to three decay modes: spontaneous fission, cluster decay, and α decay. The least action trajectory is determined in the plane (R ,η ) , where R is the separation distance of the fission fragments and η is the mass asymmetry. We may find a sequence of several trajectories one of which gives the least action. The parametrization with two deformation coordinates (R ,η ) and the radius of the light fragment, R2, exponentially or linearly decreasing with R is compared with the simpler one, in which R2=constant and with a linearly decreasing or linearly increasing R2. The latter is closer to the reality and reminds us about the α or cluster preformation at the nuclear surface.

  1. True ternary fission

    NASA Astrophysics Data System (ADS)

    Vijayaraghavan, K. R.; Balasubramaniam, M.; von Oertzen, W.

    2015-04-01

    The study of the ternary fission of nuclei has received new interest recently. It is of general interest for nuclear dynamics, although the process is very rare. In the present work, we discuss the possibilities of true ternary fission (fragment masses A >30 ) in 252Cf for different mass splits. These mass splits are strongly favored in a collinear geometry. Based on the three cluster model (TCM), it is shown that the true ternary fission into fragments with almost equal masses is one of the possible fission modes in 252Cf . For general decays it is shown that the formation of the lightest fragment at the center has the highest probability. Further the formation of tin isotopes and/or other closed shell fragments are favored. For the decay products the presence of closed shell nuclei among the three fragments enhances the decay probabilities.

  2. Radioluminescence of solid neodymium-doped laser materials excited by {alpha}-particles and fission fragments

    SciTech Connect

    Seregina, E A; Seregin, A A

    2013-02-28

    The characteristics of radioluminescence of Nd{sup 3+} : Y{sub 3}Al{sub 5}O{sub 12} crystals and laser glasses under excitation by plutonium-239 ({sup 239}Pu) {alpha}-particles, as well as by {alpha}-particles and spontaneous fission fragments of californium-252 ({sup 252}Cf), are studied. The radioluminescence branching ratios {beta}{sub ij} for the transition from the {sup 2}F2{sub 5/2} level to the {sup 2S+1}L{sub J} levels in Nd{sup 3+} : Y{sub 3}Al{sub 5}O{sub 12} crystals are measured. Radioluminescence from the {sup 2}P{sub 3/2} level to low-lying levels is observed. The {beta}{sub ij} ratios for transitions from the high-lying {sup 2}F2{sub 5/2}, {sup 4}D{sub 3/2}, and {sup 2}P{sub 3/2} levels are theoretically calculated. The lifetimes of metastable levels of Nd{sup 3+} excited by {sup 252}Cf fission fragments are measured. The efficiency of the conversion of energy of {alpha}-particles and fission fragments to the energy of optical radiation of Nd{sup 3+} : Y{sub 3}Al{sub 5}O{sub 12} crystals and laser glasses is determined. (active media)

  3. Radioluminescence of solid neodymium-doped laser materials excited by α-particles and fission fragments

    NASA Astrophysics Data System (ADS)

    Seregina, E. A.; Seregin, A. A.

    2013-02-01

    The characteristics of radioluminescence of Nd3+ : Y3Al5O12 crystals and laser glasses under excitation by plutonium-239 (239Pu) α-particles, as well as by α-particles and spontaneous fission fragments of californium-252 (252Cf), are studied. The radioluminescence branching ratios βij for the transition from the 2F25/2 level to the 2S+1LJ levels in Nd3+ : Y3Al5O12 crystals are measured. Radioluminescence from the 2P3/2 level to low-lying levels is observed. The βij ratios for transitions from the high-lying 2F25/2, 4D3/2, and 2P3/2 levels are theoretically calculated. The lifetimes of metastable levels of Nd3+ excited by 252Cf fission fragments are measured. The efficiency of the conversion of energy of α-particles and fission fragments to the energy of optical radiation of Nd3+ : Y3Al5O12 crystals and laser glasses is determined.

  4. Novel Scintillation Detectors for Prompt Fission γ-Ray Measurements

    NASA Astrophysics Data System (ADS)

    Billnert, R.; Andreotti, E.; Hambsch, F.-J.; Hult, M.; Karlsson, J.; Marissens, G.; Oberstedt, A.; Oberstedt, S.

    In this work we present first results from measurements of prompt fission γ-rays from the spontaneous fission in 252Cf. New and accurate data on corresponding γ-rays from the reactions 235U(nth,f) and 239Pu(nth,f) are highly demanded for the modeling of new Generation-IV nuclear reactor systems. For these experiments we employed scintillation detectors made out of new materials (LaBr3, LaCl3 and CeBr3), whose properties were necessary to know in order to obtain reliable results. Hence, we have characterized these detectors. In all the important properties these detectors outshine sodium-iodine detectors that where used in the 1970s, when the existing data had been acquired. Our finding is that the new generation of scintillation detectors is indeed promising, as far as an improved precision of the demanded data is concerned.

  5. Ground state spontaneous fission half-lives from thorium to fermium

    SciTech Connect

    Holden, N.E.

    1988-01-01

    Measurements of the half-lives for spontaneous fission of the nuclidic ground states of elements from thorium to fermium have been compiled and evaluated. Recommended values are presented. An attempt has been made to distinguish between spontaneous fission and heavy ion emission. Spontaneously fissioning isomers have not been considered here. The difference between even-even nuclides and odd-even, even-odd and odd-odd nuclides are discussed. 3 tabs.

  6. Coincident measurements of prompt fission γ rays and fission fragments at DANCE

    NASA Astrophysics Data System (ADS)

    Walker, C. L.; Baramsai, B.; Jandel, M.; Rusev, G.; Couture, A.; Mosby, S.; Ullmann, J.; Kawano, T.; Stetcu, I.; Talou, P.

    2015-10-01

    Modern statistical approaches to modeling fission involve the calculation of not only average quantities but also fully correlated distributions of all fission products. Applications such as those involving the detection of special nuclear materials also rely on fully correlated data of fission products. Experimental measurements of correlated data are thus critical to the validation of theory and the development of important applications. The goal of this experiment was to measure properties of prompt fission gamma-ray emission as a function of fission fragments' total kinetic energy in the spontaneous fission of 252Cf. The measurement was carried out at the Detector for Advanced Neutron Capture Experiments (DANCE), a 4 π γ-ray calorimeter. A prototype design consisting of two silicon detectors was installed in the center of DANCE, allowing simultaneous measurement of fission fragments and γ rays. Effort has been taken to simulate fragment kinetic energy losses as well as γ-ray attenuation in DANCE using such tools as GEANT4 and SRIM. Theoretical predictions generated by the code CGMF were also incorporated as input for these simulations. Results from the experiment and simulations will be presented, along with plans for future measurements.

  7. In-beam gamma-ray spectroscopy of {sup 248,250,252}Cf by neutron-transfer reactions using a Cf target

    SciTech Connect

    Takahashi, R.; Ishii, T.; Asai, M.; Nagae, D.; Makii, H.; Tsukada, K.; Toyoshima, A.; Ishii, Y.; Matsuda, M.; Makishima, A.; Shizuma, T.; Kohno, T.; Ogawa, M.

    2010-05-15

    The ground-state bands of {sup 248,250,252}Cf have been established up to the 10{sup +}, 12{sup +}, and 10{sup +} states, respectively, by in-beam gamma-ray spectroscopy using neutron-transfer reactions with a 153-MeV {sup 18}O beam and a highly radioactive Cf target. The deexcitation gamma rays in {sup 248,250,252}Cf were identified by taking coincidences with outgoing particles of {sup 16-19}O measured with Si DELTAE-E detectors, and by selecting their kinetic energies. Moments of inertia of {sup 248,250,252}Cf were discussed in terms of the N=152 deformed shell gap.

  8. Microscopic modeling of mass and charge distributions in the spontaneous fission of 240Pu

    NASA Astrophysics Data System (ADS)

    Sadhukhan, Jhilam; Nazarewicz, Witold; Schunck, Nicolas

    2016-01-01

    We propose a methodology to calculate microscopically the mass and charge distributions of spontaneous fission yields. We combine the multidimensional minimization of collective action for fission with stochastic Langevin dynamics to track the relevant fission paths from the ground-state configuration up to scission. The nuclear potential energy and collective inertia governing the tunneling motion are obtained with nuclear density functional theory in the collective space of shape deformations and pairing. We obtain a quantitative agreement with experimental data and find that both the charge and mass distributions in the spontaneous fission of 240Pu are sensitive both to the dissipation in collective motion and to adiabatic fission characteristics.

  9. Future research program on prompt γ-ray emission in nuclear fission

    NASA Astrophysics Data System (ADS)

    Oberstedt, S.; Billnert, R.; Hambsch, F.-J.; Lebois, M.; Oberstedt, A.; Wilson, J. N.

    2015-12-01

    In recent years the measurement of prompt fission γ-ray spectra (PFGS) has gained renewed interest, after about forty years since the first comprehensive studies of the reactions 235U(n th , f), 239Pu(n th ,f) and 252Cf(sf). The renaissance was initiated by requests for new values especially for γ-ray multiplicity and average total energy release per fission in neutron-induced fission of 235U and 239Pu. Both isotopes are considered the most important ones with respect to the modeling of innovative cores required for the Generation-IV reactors, the majority working with fast neutrons. During the last 5 years we have conducted a systematic study of spectral data for thermal-neutron-induced fission on 235U and 241Pu as well as for the spontaneous fission of 252Cf with unprecedented accuracy. From the new data we conclude that those reactions do not considerably contribute to the observed heat excess and suspect other reactions playing a significant role. Possible contributions may originate from fast-neutron-induced reactions on 238U, which is largely present in the fuel, or from γ-induced fission from neutron capture in the construction material. A first experiment campaign on prompt γ-ray emission from fast-neutron-induced fission on 235,238U was successfully performed in order to test our assumptions. In the following we attempt to summarize, what has been done in the field to date, and to motivate future measurement campaigns exploiting dedicated neutron and photon beams as well as upcoming highly efficient detector assemblies.

  10. The Spontaneous Mutation Rate in the Fission Yeast Schizosaccharomyces pombe.

    PubMed

    Farlow, Ashley; Long, Hongan; Arnoux, Stéphanie; Sung, Way; Doak, Thomas G; Nordborg, Magnus; Lynch, Michael

    2015-10-01

    The rate at which new mutations arise in the genome is a key factor in the evolution and adaptation of species. Here we describe the rate and spectrum of spontaneous mutations for the fission yeast Schizosaccharomyces pombe, a key model organism with many similarities to higher eukaryotes. We undertook an ∼1700-generation mutation accumulation (MA) experiment with a haploid S. pombe, generating 422 single-base substitutions and 119 insertion-deletion mutations (indels) across the 96 replicates. This equates to a base-substitution mutation rate of 2.00 × 10(-10) mutations per site per generation, similar to that reported for the distantly related budding yeast Saccharomyces cerevisiae. However, these two yeast species differ dramatically in their spectrum of base substitutions, the types of indels (S. pombe is more prone to insertions), and the pattern of selection required to counteract a strong AT-biased mutation rate. Overall, our results indicate that GC-biased gene conversion does not play a major role in shaping the nucleotide composition of the S. pombe genome and suggest that the mechanisms of DNA maintenance may have diverged significantly between fission and budding yeasts. Unexpectedly, CpG sites appear to be excessively liable to mutation in both species despite the likely absence of DNA methylation.

  11. The Spontaneous Mutation Rate in the Fission Yeast Schizosaccharomyces pombe

    PubMed Central

    Farlow, Ashley; Long, Hongan; Arnoux, Stéphanie; Sung, Way; Doak, Thomas G.; Nordborg, Magnus; Lynch, Michael

    2015-01-01

    The rate at which new mutations arise in the genome is a key factor in the evolution and adaptation of species. Here we describe the rate and spectrum of spontaneous mutations for the fission yeast Schizosaccharomyces pombe, a key model organism with many similarities to higher eukaryotes. We undertook an ∼1700-generation mutation accumulation (MA) experiment with a haploid S. pombe, generating 422 single-base substitutions and 119 insertion-deletion mutations (indels) across the 96 replicates. This equates to a base-substitution mutation rate of 2.00 × 10−10 mutations per site per generation, similar to that reported for the distantly related budding yeast Saccharomyces cerevisiae. However, these two yeast species differ dramatically in their spectrum of base substitutions, the types of indels (S. pombe is more prone to insertions), and the pattern of selection required to counteract a strong AT-biased mutation rate. Overall, our results indicate that GC-biased gene conversion does not play a major role in shaping the nucleotide composition of the S. pombe genome and suggest that the mechanisms of DNA maintenance may have diverged significantly between fission and budding yeasts. Unexpectedly, CpG sites appear to be excessively liable to mutation in both species despite the likely absence of DNA methylation. PMID:26265703

  12. A feasibility study of [sup 252]Cf neutron brachytherapy, cisplatin + 5-FU chemo-adjuvant and accelerated hyperfractionated radiotherapy for advanced cervical cancer

    SciTech Connect

    Murayama, Y.; Wierzbicki, J. Univ. of Kentucky Medical Center, Lexington, KY ); Bowen, M.G.; Van Nagell, J.R.; Gallion, H.H.; DePriest, P. )

    1994-06-15

    The purpose was to evaluate the feasibility and toxicity of [sup 252]Cf neutron brachytherapy combined with hyperaccelerated chemoradiotherapy for Stage III and IV cervical cancers. Eleven patients with advanced Stage IIIB-IVA cervical cancers were treated with [sup 252]Cf neutron brachytherapy in an up-front schedule followed by cisplatin (CDDP; 50 mg/m[sup 2]) chemotherapy and hyperfractionated accelerated (1.2 Gy bid) radiotherapy given concurrently with intravenous infusion of 5-Fluorouracil (5-FU) (1000 mg/m[sup 2]/day [times] 4 days) in weeks 1 and 4 with conventional radiation (weeks 2, 3, 5, and 6). Total dose at a paracervical point A isodose surface was 80-85 Gy-eq by external and intracavitary therapy and 60 Gy at the pelvic sidewalls. Patients tolerated the protocol well. There was 91% compliance with the chemotherapy and full compliance with the [sup 252]Cf brachytherapy and the external beam radiotherapy. There were no problems with acute chemo or radiation toxicity. One patient developed a rectovaginal fistula (Grade 3-4 RTOG criteria) but no other patients developed significant late cystitis, proctitis or enteritis. There was complete response (CR) observed in all cases. With mean follow-up to 26 months, local control has been achieved with 90% actuarial 3-year survival with no evidence of disease (NED). [sup 252]Cf neutrons can be combined with cisplatin and 5-FU infusion chemotherapy plus hyperaccelerated chemoradiotherapy without unusual side effects or toxicity and with a high local response and tumor control rate. Further study of [sup 252]Cf neutron-chemoradiotherapy for advanced and bulky cervical cancer are indicated. The authors found chemotherapy was more effective with the improved local tumor control. 18 refs., 2 tabs.

  13. Fission properties of the 1. 5-s spontaneous fission activity produced in bombardmentof /sup 248/Cm with /sup 18/O

    SciTech Connect

    Hoffman, D.C.; Lee, D.; Ghiorso, A.; Nurmia, M.J.; Aleklett, K.; Leino, M.

    1981-08-01

    We have measured the mass and kinetic-energy distributions of fragments from the spontaneous fission of a 1.5-s activity produced in bombardments of /sup 248/Cm with 95-MeV /sup 18/O ions. Its spontaneous fission decay exhibits a very symmetric, narrow (full width at half maximum = 12 mass units) mass distribution, a very high total kinetic energy of 234 +- 2 MeV, and increasing total kinetic energy with increasingly symmetric mass division. Based on its half-life and the similarity of its fission properties to the unique fission properties so far only observed for /sup 258/Fm and /sup 259/Fm, the most likely assignment of this activity is to the known /sup 259/Fm. However, assignment to some as yet undiscovered neutron-rich heavy element isotope such as /sup 260/Md cannot be unequivocally excluded.

  14. A double-Bragg detector with digital signal processing for the event-by-event study of fission in actinide nuclei

    NASA Astrophysics Data System (ADS)

    Frost, R. J. W.; Smith, A. G.

    2016-09-01

    In the current paper, a windowless double-Bragg chamber incorporating full signal digitisation has been developed for the purpose of studying the energy (E), mass (A), charge (Z) and angular distributions (θ, Φ) of nuclei generated by fission. This device measures E for each fission fragment by collection of the charge produced during ionisation of the fill gas. Subsequent digitisation of the signals from each of two anodes yields information on dE/dx, as well as electron collection time, which can be further used for polar angle (θ) determination. Frisch-grid and cathode signals are also digitised and are used both for anode signal correction and to produce further information on θ. To verify the operation of this detector, three angular determination techniques from the literature were implemented, and the results were found to be consistent with the referenced paper. Current results from the spontaneous fission of 252Cf are presented.

  15. Measurement of Neutron Induced and Spontaneous Fission in Pu-242 at DANCE

    NASA Astrophysics Data System (ADS)

    Chyzh, Andrii; Wu, C. Y.; Henderson, R.; Couture, A.; Lee, H. Y.; Ullmann, J.; O'Donnell, J. M.; Jandel, M.; Haight, R. C.; Bredeweg, T. A.; Dance Collaboration

    2013-10-01

    Neutron capture and fission reactions are important in nuclear engineering and physics. DANCE (Detector for Advanced Neutron Capture Measurement, LANL) combined with PPAC (avalanche technique based fission tagging detector, LLNL) were used to study neutron induced and spontaneous fission in 242Pu. 2 measurements were performed in 2013. The first experiment was done without the incident neutron beam with the fission tagging ability to study γ-rays emitted in the spontaneous fission of 242Pu. The second one - with the neutron beam to measure both the neutron capture and fission reactions. This is the first direct measurement of prompt fission γ-rays in 242Pu. The γ-ray multiplicity, γ-ray energy, and total energy of γ-rays per fission in 242Pu will be presented. These distributions of the 242Pu spontaneous fission will be compared to those in the 241Pu neutron induced fission. This work was performed under the auspices of the US Department of Energy by Los Alamos National Laboratory under Contract DE-AC52-06NA25396 and Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

  16. Search for instantaneous radiation near the instant of break momentum of various fissioning nuclear systems at low excitation energies

    SciTech Connect

    Vorobyev, A. S. Val'ski, G. V.; Gagarskii, A. M.; Guseva, I. S.; Petrov, G. A.; Petrova, V. I.; Serebrin, A. Yu.; Sokolov, V. E.; Shcherbakov, O. A.

    2011-12-15

    The main results of studying the properties of 'instantaneous' neutrons and {gamma} photons during the fission of {sup 233,235}U(n{sub th}, f) and {sup 239}Pu(n{sub th}, f) nuclei and spontaneous fission of {sup 252}Cf, which were performed on the WWR-M reactor at the St. Petersburg Nuclear Physics Institute, Russian Academy of Sciences, are presented. Along with obtaining the main characteristics of the instantaneous radiation from fission fragments, these studies were also aimed at gaining deeper insight into such exotic processes as the emission of break neutrons and {gamma} photons from a fissioning nucleus near the break point. These investigations were performed on different experimental setups using different analytical methods. This approach allowed us not only to find but also to reduce to minimum possible systematic effects. The yields of break neutrons were found to be about (5-7) Multiplication-Sign 10{sup -2} of the total number of neutrons per {sup 233,235}U(n, f) fission event and approximately twice as much for {sup 239}Pu(n, f) and {sup 252}Cf. The coefficient of T-odd asymmetry for {gamma} photons is in agreement with the estimate obtained on the assumption that the observed effect is mainly related to the {gamma} photons emitted by excited fragments with highly oriented angular momenta. This fact gave grounds to conclude that the desired break {gamma} photons cannot be reliably selected (within the obtained experimental accuracy) against the much larger background of {gamma} photons from fission fragments.

  17. Benchmark Experiments of Thermal Neutron and Capture Gamma-Ray Distributions in Concrete Using {sup 252}Cf

    SciTech Connect

    Asano, Yoshihiro; Sugita, Takeshi; Hirose, Hideyuki; Suzaki, Takenori

    2005-10-15

    The distributions of thermal neutrons and capture gamma rays in ordinary concrete were investigated by using {sup 252}Cf. Two subjects are considered. One is the benchmark experiments for the thermal neutron and the capture gamma-ray distributions in ordinary concrete. The thermal neutron and the capture gamma-ray distributions were measured by using gold-foil activation detectors and thermoluminescence detectors. These were compared with the simulations by using the discrete ordinates code ANISN with two different group structure types of cross-section library of a new Japanese version, JENDL-3.3, showing reasonable agreement with both fine and rough structure groups of thermal neutron energy. The other is a comparison of the simulations with two different cross-section libraries, JENDL-3.3 and ENDF/B-VI, for the deep penetration of neutrons in the concrete, showing close agreement in 0- to 100-cm-thick concrete. However, the differences in flux grow with an increase in concrete thickness, reaching up to approximately eight times near 4-m thickness.

  18. Properties of true quaternary fission of nuclei with allowance for its multistep and sequential character

    SciTech Connect

    Kadmensky, S. G. Titova, L. V.; Bulychev, A. O.

    2015-07-15

    An analysis of basicmechanisms of binary and ternary fission of nuclei led to the conclusion that true ternary and quaternary fission of nuclei has a sequential two-step (three-step) character, where, at the first step, a fissile nucleus emits a third light particle (third and fourth light particles) under shakeup effects associated with a nonadiabatic character of its collective deformation motion, whereupon the residual nucleus undergoes fission to two fission fragments. Owing to this, the formulas derived earlier for the widths with respect to sequential two- and three-step decays of nuclei in constructing the theory of two-step twoproton decays and multistep decays in chains of genetically related nuclei could be used to describe the relative yields and angular and energy distributions of third and fourth light particles emitted in (α, α), (t, t), and (α, t) pairs upon the true quaternary spontaneous fission of {sup 252}Cf and thermal-neutron-induced fission of {sup 235}U and {sup 233}U target nuclei. Mechanisms that explain a sharp decrease in the yield of particles appearing second in time and entering into the composition of light-particle pairs that originate from true quaternary fission of nuclei in relation to the yields of analogous particles in true ternary fission of nuclei are proposed.

  19. Properties of true quaternary fission of nuclei with allowance for its multistep and sequential character

    NASA Astrophysics Data System (ADS)

    Kadmensky, S. G.; Titova, L. V.; Bulychev, A. O.

    2015-07-01

    An analysis of basicmechanisms of binary and ternary fission of nuclei led to the conclusion that true ternary and quaternary fission of nuclei has a sequential two-step (three-step) character, where, at the first step, a fissile nucleus emits a third light particle (third and fourth light particles) under shakeup effects associated with a nonadiabatic character of its collective deformation motion, whereupon the residual nucleus undergoes fission to two fission fragments. Owing to this, the formulas derived earlier for the widths with respect to sequential two- and three-step decays of nuclei in constructing the theory of two-step twoproton decays and multistep decays in chains of genetically related nuclei could be used to describe the relative yields and angular and energy distributions of third and fourth light particles emitted in ( α, α), ( t, t), and ( α, t) pairs upon the true quaternary spontaneous fission of 252Cf and thermal-neutron-induced fission of 235U and 233U target nuclei. Mechanisms that explain a sharp decrease in the yield of particles appearing second in time and entering into the composition of light-particle pairs that originate from true quaternary fission of nuclei in relation to the yields of analogous particles in true ternary fission of nuclei are proposed.

  20. Microscopic modeling of mass and charge distributions in the spontaneous fission of 240Pu

    DOE PAGES

    Sandhukhan, Jhilam; Nazarewicz, Witold; Schunck, Nicolas

    2016-01-20

    We propose a methodology to calculate microscopically the mass and charge distributions of spontaneous fission yields. We combine the multidimensional minimization of collective action for fission with stochastic Langevin dynamics to track the relevant fission paths from the ground-state configuration up to scission. The nuclear potential energy and collective inertia governing the tunneling motion are obtained with nuclear density functional theory in the collective space of shape deformations and pairing. As a result, we obtain a quantitative agreement with experimental data and find that both the charge and mass distributions in the spontaneous fission of 240Pu are sensitive both tomore » the dissipation in collective motion and to adiabatic fission characteristics.« less

  1. Shielding evaluation of a medical linear accelerator vault in preparation for installing a high-dose rate 252Cf remote afterloader.

    PubMed

    Melhus, C S; Rivard, M J; Kurkomelis, J; Liddle, C B; Massé, F X

    2005-01-01

    In support of the effort to begin high-dose rate 252Cf brachytherapy treatments at Tufts-New England Medical Center, the shielding capabilities of a clinical accelerator vault against the neutron and photon emissions from a 1.124 mg 252Cf source were examined. Outside the clinical accelerator vault, the fast neutron dose equivalent rate was below the lower limit of detection of a CR-39 etched track detector and below 0.14 +/- 0.02 muSv h(-1) with a proportional counter, which is consistent, within the uncertainties, with natural background. The photon dose equivalent rate was also measured to be below background levels (0.1 muSv h(-1)) using an ionisation chamber and an optically stimulated luminescence dosemeter. A Monte Carlo simulation of neutron transport through the accelerator vault was performed to validate measured values and determine the thermal-energy to low-energy neutron component. Monte Carlo results showed that the dose equivalent rate from fast neutrons was reduced by a factor of 100,000 after attenuation through the vault wall, and the thermal-energy neutron dose equivalent rate would be an additional factor of 1000 below that of the fast neutrons. Based on these findings, the shielding installed in this facility is sufficient for the use of at least 5.0 mg of 252Cf.

  2. Event-by-event study of neutron observables in spontaneous and thermal fission

    SciTech Connect

    Vogt, R; Randrup, J

    2011-09-14

    The event-by-event fission model FREYA is extended to spontaneous fission of actinides and a variety of neutron observables are studied for spontaneous fission and fission induced by thermal neutrons with a view towards possible applications for SNM detection. We have shown that event-by-event models of fission, such as FREYA, provide a powerful tool for studying fission neutron correlations. Our results demonstrate that these correlations are significant and exhibit a dependence on the fissioning nucleus. Since our method is phenomenological in nature, good input data are especially important. Some of the measurements employed in FREYA are rather old and statistics limited. It would be useful to repeat some of these studies with modern detector techniques. In addition, most experiments made to date have not made simultaneous measurements of the fission products and the prompt observables, such as neutron and photons. Such data, while obviously more challenging to obtain, would be valuable for achieving a more complete understanding of the fission process.

  3. Second malignancies following conventional or combined 252Cf neutron brachytherapy with external beam radiotherapy for breast cancer

    PubMed Central

    Valuckas, Konstantinas Povilas; Atkocius, Vydmantas; Kuzmickiene, Irena; Aleknavicius, Eduardas; Liukpetryte, Sarune; Ostapenko, Valerijus

    2013-01-01

    We retrospectively evaluated the risk of second malignancies among 832 patients with inner or central breast cancer treated with conventional external beam schedule (CRT group), or neutron brachytherapy using Californium-252 (252Cf) sources and hypofractionated external beam radiotherapy (HRTC group), between 1987 and 1996 at the Institute of Oncology, Vilnius University. Patients were observed until the occurrences of death or development of a second malignancy, or until 31 December 2009, whichever was earlier. Median follow-up time was 10.4 years (range, 1.2–24.1 years). Risk of second primary cancers was quantified using standardized incidence ratios (SIRs). Cox proportional hazards regression models were used to estimate hazard ratios (HRs). There was a significant increase in the risk of second primary cancers compared with the general population (SIR 1.3, 95% CI 1.1–1.5). The observed number of second primary cancers was also higher than expected for breast (SIR 1.8, 95% CI 1.3–2.4) and lung cancer (SIR 3.8, 95% CI 2.0–6.7). For second breast cancer, no raised relative risk was observed during the period ≥10 or more years after radiotherapy. Compared with the CRT group, HRTC patients had a not statistically significant higher risk of breast cancer. Increased relative risks were observed specifically for age at initial diagnosis of <50 years (HR 2.9, 95% CI 1.6–5.2) and for obesity (HR 2.8, 95% CI 1.1–7.2). PMID:23397075

  4. Prompt neutron emission from the spontaneous fission of sup 260 Md

    SciTech Connect

    Wild, J.F.; van Aarle, J.; Westmeier, W.; Lougheed, R.W.; Hulet, E.K.; Moody, K.J.; Dougan, R.J.; Koop, E.; Glaser, R.E.; Brandt, R.; Patzelt, P. Philipps University, D-3550, Marburg an der Lahn, )

    1990-02-01

    We have made the first measurement of the number of neutrons emitted from the spontaneous fission of a nuclide in which very high fragment energies dominate the fission process. In bombardments of {sup 254}Es, we produced a large sample of 28-d {sup 260}Md, which was neutron counted in a 1-m-diameter spherical tank containing a Gd-doped scintillator solution. The average number of neutrons emitted per fission is only 2.58{plus minus}0.11, substantially less than for other actinides. A linear dependence of neutron multiplicity on fragment-excitation energy is observed to the highest values of total kinetic energy.

  5. Neutron emission as a function of fragment energy in the spontaneous fission of /sup 260/Md

    SciTech Connect

    Wild, J.F.; van Aarle, J.; Westmeiser, W.; Lougheed, R.W.; Hulet, E.K.; Moody, K.J.; Dougan, R.J.; Brandt, R.; Patzelt, P.

    1989-04-19

    We have made the first measurement of the number of neutrons emitted in the spontaneous fission of a nuclide in which very high fragment energies dominate the fission process. In bombardments of /sup 254/Es, we produced 28-d /sup 260/Md, which was neutron-counted in a 1-m-diam spherical tank containing a Gd-doped scintillator solution. The average number of neutrons emitted per fission is only 2.58 +- 0.11, substantially less than for other actinides. A direct correlation of neutron multiplicity with fragment excitation energy is clearly demonstrated. 3 refs., 5 figs.

  6. Even-odd effects in prompt emission of spontaneously fissioning even-even Pu isotopes

    NASA Astrophysics Data System (ADS)

    Tudora, A.; Hambsch, F.-J.; Giubega, G.; Visan, I.

    2015-01-01

    The available experimental Y (A , TKE) data for 236,238,240,242,244Pu(SF) together with the Zp model prescription with appropriate parameters allows the investigation of even-odd effects in fragment distributions. The size of the global even-odd effect in Y (Z) is decreasing from 244Pu(SF) to 236Pu(SF) confirming the general observation of a decrease of the even-odd effect with the fissility parameter. Charge polarizations (ΔZ) and root-mean squares (rms) as a function of A of 236-244Pu(SF) were obtained for the first time. In the asymmetric fission region both ΔZ (A) and rms (A) exhibit oscillations with a periodicity of about 5 mass units due to the even-odd effects. The total average charge deviations < ΔZ > (obtained by averaging ΔZ (A) over the experimental Y (A) distribution) are of about |0.5| for all studied Pu(SF) systems. The comparison of the calculated ΔZ (A) and rms (A) of 240Pu(SF) with those of 239Pu (nth , f) reported by Wahl shows an in-phase oscillation with a higher amplitude in the case of 240Pu(SF), confirming the higher even-odd effect in the case of SF. As in the previously studied cases (233,235U (nth , f), 239Pu (nth , f), 252Cf(SF)) the even-odd effects in the prompt emission of 236-244Pu(SF) are mainly due to the Z even-odd effects in fragment distributions and charge polarizations and the N even-odd effects in the average neutron separation energies from fragments < Sn >. The size of the global N even-odd effect in < Sn > is decreasing with the fissility parameter, being higher for the Pu(SF) systems compared to the previously studied systems. The prompt neutron multiplicities as a function of Z, ν (Z), exhibit sawtooth shapes with a visible staggering for asymmetric fragmentations. The size of the global Z even-odd effect in ν (Z) exhibits a decreasing trend with increasing fissility. The average prompt neutron multiplicities as a function of TKE show an increase of the even-odd effect with increasing TKE, with global effect

  7. Development of a thin scintillation films fission-fragment detector and a novel neutron source

    NASA Astrophysics Data System (ADS)

    Rusev, G.; Jandel, M.; Baramsai, B.; Bond, E. M.; Bredeweg, T. A.; Couture, A.; Daum, J. K.; Favalli, A.; Ianakiev, K. D.; Iliev, M. L.; Mosby, S.; Roman, A. R.; Springs, R. K.; Ullmann, J. L.; Walker, C. L.

    2015-08-01

    Investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flight spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

  8. Development of a thin scintillation films fission-fragment detector and a novel neutron source

    DOE PAGES

    Rusev, Gencho Yordanov; Jandel, Marian; Baramsai, Bayarbadrakh; Bond, Evelyn M.; Bredeweg, Todd Allen; Couture, Aaron Joseph; Daum, Jaimie Kay; Favalli, Andrea; Ianakiev, Kiril Dimitrov; Iliev, Metodi L.; et al

    2015-08-26

    Here, investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flightmore » spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.« less

  9. Microarray analysis of DNA damage repair gene expression profiles in cervical cancer cells radioresistant to 252Cf neutron and X-rays

    PubMed Central

    2010-01-01

    Background The aim of the study was to obtain stable radioresistant sub-lines from the human cervical cancer cell line HeLa by prolonged exposure to 252Cf neutron and X-rays. Radioresistance mechanisms were investigated in the resulting cells using microarray analysis of DNA damage repair genes. Methods HeLa cells were treated with fractionated 252Cf neutron and X-rays, with a cumulative dose of 75 Gy each, over 8 months, yielding the sub-lines HeLaNR and HeLaXR. Radioresistant characteristics were detected by clone formation assay, ultrastructural observations, cell doubling time, cell cycle distribution, and apoptosis assay. Gene expression patterns of the radioresistant sub-lines were studied through microarray analysis and verified by Western blotting and real-time PCR. Results The radioresistant sub-lines HeLaNR and HeLaXR were more radioresisitant to 252Cf neutron and X-rays than parental HeLa cells by detecting their radioresistant characteristics, respectively. Compared to HeLa cells, the expression of 24 genes was significantly altered by at least 2-fold in HeLaNR cells. Of these, 19 genes were up-regulated and 5 down-regulated. In HeLaXR cells, 41 genes were significantly altered by at least 2-fold; 38 genes were up-regulated and 3 down-regulated. Conclusions Chronic exposure of cells to ionizing radiation induces adaptive responses that enhance tolerance of ionizing radiation and allow investigations of cellular radioresistance mechanisms. The insights gained into the molecular mechanisms activated by these "radioresistance" genes will lead to new therapeutic targets for cervical cancer. PMID:20184742

  10. Multidimensional Skyrme-density-functional study of the spontaneous fission of 238U

    SciTech Connect

    Sadhukhan, J.; Mazurek, K.; Dobaczewski, J.; Nazarewicz, W.; Sheikh, J. A.; Baran, A.

    2015-01-01

    We determined the spontaneous fission lifetime of 238U by a minimization of the action integral in a three-dimensional space of collective variables. Apart from the mass-distribution multipole moments Q20 (elongation) and Q30 (left–right asymmetry), we also considered the pairing-fluctuation parameter λ2 as a collective coordinate. The collective potential was obtained self-consistently using the Skyrme energy density functional SkM*. The inertia tensor was obtained within the nonperturbative cranking approximation to the adiabatic time-dependent Hartree–Fock–Bogoliubov approach. As a result, the pairing-fluctuation parameter λ2 allowed us to control the pairing gap along the fission path, which significantly changed the spontaneous fission lifetime.

  11. Multidimensional Skyrme-density-functional study of the spontaneous fission of 238U

    DOE PAGES

    Sadhukhan, J.; Mazurek, K.; Dobaczewski, J.; Nazarewicz, W.; Sheikh, J. A.; Baran, A.

    2015-01-01

    We determined the spontaneous fission lifetime of 238U by a minimization of the action integral in a three-dimensional space of collective variables. Apart from the mass-distribution multipole moments Q20 (elongation) and Q30 (left–right asymmetry), we also considered the pairing-fluctuation parameter λ2 as a collective coordinate. The collective potential was obtained self-consistently using the Skyrme energy density functional SkM*. The inertia tensor was obtained within the nonperturbative cranking approximation to the adiabatic time-dependent Hartree–Fock–Bogoliubov approach. As a result, the pairing-fluctuation parameter λ2 allowed us to control the pairing gap along the fission path, which significantly changed the spontaneous fission lifetime.

  12. Role of the second barrier upon mass division in the spontaneous fission of the heaviest elements

    SciTech Connect

    Hulet, E.K. )

    1994-07-01

    In the region where theorists had earlier predicted the disappearance of the outer fission barrier or its dropping below the ground state, the mass and total kinetic-energy distributions from spontaneous fission of [sup 252]No, [sup 254]No, [sup 256][104], and [sup 258][104] have been measured. The results, in combination with earlier measurements for [sup 256]No, [sup 258]No, and [sup 262]No, show a sharp transition from the asymmetrical mass division in [sup 256]No to the symmetrical mass division for [sup 258]No and [sup 262]No. Conversely, all isotopes of element 104, including [sup 260][104], appear to yield broadly symmetrical mass distributions. The total kinetic energies around 200 MeV for the 104 isotopes indicate the fission by the low-energy mode of bimodal fission. Based on the hypothesis that the second barrier is responsible for the asymmetrical mass distributions, and when it disappears, for symmetrical ones, these observations for the isotopes of element 104 are in agreement with the 1976 calculations of the heights of the second fission barrier relative to the ground state. Some recent calculations of static potential-energy surfaces and of barrier heights deduced from half lives for spontaneous fission indicate that the second barrier is from 0 to 2.9 MeV above the ground state for the No and 104 isotopes. However, shape degrees of freedom have been limited in these calculations; therefore, they fail to provide realistic heights for the outer fission barrier. For the few cases where higher-order asymmetrical deformations are included, this barrier height is well below the ground state and, for these nuclides, symmetrical mass division only is observed. Without more extensive calculations of potential-energy surfaces for comparison with the findings, a firm conclusion about the role of the second barrier upon mass division in fission is impossible to obtain.

  13. Role of the second barrier upon mass division in the spontaneous fission of the heaviest elements

    SciTech Connect

    Hulet, E.K.

    1993-10-01

    In the region where theorists had earlier predicted the disappearance of the outer fission barrier or of it dropping below the ground-state, we have measured the mass and total-kinetic-energy distributions from spontaneous fission of {sup 252}No, {sup 254}No, {sup 256}[104], and {sup 258}[104]. The results, in combination with earlier measurements for {sup 256}No, {sup 258}No, and {sup 262}No, show a sharp transition from asymmetrical mass division in {sup 256}No to symmetrical ones for {sup 258}No and {sup 262}No. On-the-other-hand, all isotopes of element 104 including {sup 260}[104] appear to yield broadly symmetrical mass distributions. The total-kinetic energies around 200 MeV for the 104 isotopes indicate they fission by the low-energy mode of bimodal fission. Based on the hypothesis that the second barrier is responsible for asymmetrical mass distributions and when it disappears, for symmetrical ones, these observations for the isotopes of element 104 are in accord with 1976 calculations of the heights of the second fission barrier relative to the ground-state. Some recent calculations of static potential-energy surfaces and of barrier heights deduced from half-lives for spontaneous fission indicate the second barrier is from 0 to 2.9 MeV above the ground-state for the No and 104 isotopes. However, shape degrees-of-freedom have been limited in these calculations so that they fail to provide realistic heights for the outer fission barrier. For the few cases where higher-order asymmetrical deformations are included, this barrier height is well below the ground-state and, for these nuclides, we observe symmetric mass division only. Without more extensive calculations of potential-energy surfaces for comparison with our findings, we are unable reach a firm conclusion on the role of the second barrier upon mass division in fission.

  14. QUALIFICATION OF THE SAVANNAH RIVER SITE 252CF SHUFFLER FOR RECEIPT VERIFICATION MEASUREMENTS OF MIXED U-PU OXIDES STORED IN 9975 SHIPPING CONTAINERS

    SciTech Connect

    Dubose, F.

    2011-05-26

    To extend their ability to perform accountability and verification measurements of {sup 235}U in a U-Pu oxide matrix, the K-Area Material Storage facility commissioned the development and construction of a Passive/Active {sup 252}Cf Shuffler. A series of {sup 252}Cf, PuO{sub 2}, and U-Pu oxide standards, in addition to a single U{sub 3}O{sub 8} standard, were measured to characterize and calibrate the shuffler. Accompanying these measurements were simulations using MCNP5/MCNPX, aimed at isolating the neutron countrate contributions for each of the isotopes present. Two calibration methods for determining the {sup 235}U content in mixed UPu oxide were then developed, yielding comparable results. The first determines the {sup 235}U mass by estimating the {sup 239}Pu/{sup 235}U ratio-dependent contributions from the primary delayed neutron contributors. The second defines an average linear response based on the {sup 235}U and {sup 239}Pu mass contents. In each case, it was observed that self-shielding due to {sup 235}U mass has a large influence on the observed rates, requiring bounds on the applicable limits of each calibration method.

  15. Development of Two-Dimensional Fitting and Application to Prompt Gamma-Rays of CALIFORNIUM-252 Fission

    NASA Astrophysics Data System (ADS)

    Chemaly, Mike Georges

    We have developed a method for the direct two -dimensional decomposition of complex coincidence matrices in order to extract gamma-gamma coincidence intensities at the statistical limits. The algorithms written to analyze the gamma-gamma coincidence data were developed first while working on unidimensional spectra from the decay of ^ {65}Ni, ^{65} Zn and ^{rm 108m} Ag. They were then extended to work in two dimensions in order to obtain a general method that could be used for extracting information from data sets having different dimensions. We successfully modeled the continuum and the ridges over the entire coincidence matrix. The continuum is described by the simple product of two vectors while the ridges are reproduced from a centroid based on gamma -rays in the total projection and a vector giving the height as a function of position. The peaks found by a two-dimensional zero-area transform are fitted with a Singular Value Decomposition --Levenberg Marquardt code extended to two dimensions. We applied the technique to the analysis of the coincidences involving the prompt gammas from the spontaneous fission of ^{252}Cf. The information from the 20,000 coincidence peaks obtained from the fit was manipulated through a computer program. The built-in database constructed from NNDC nuclear structure data files provided access to literature schemes. A graphical interface allowed the interactive building and extension of level schemes. Newly placed transitions were checked by comparing predicted coincidences to those observed. In the even-even nuclides, models like the Variable-Moment -of-Inertia and the product of valence protons and neutrons (NpNn scheme) are used to guide placements based on systematics. We take advantage of the cross-coincidences between fission partners to determine the atomic number and mass of the nuclide in which a transition occurred. Fifty-eight level schemes from ^{252}Cf fission have been constructed and seventeen of them have been

  16. Development of position-sensitive time-of-flight spectrometer for fission fragment research

    SciTech Connect

    Arnold, C. W.; Tovesson, F.; Meierbachtol, K.; Bredeweg, T.; Jandel, M.; Jorgenson, H. J.; Laptev, A.; Rusev, G.; Shields, D. W.; White, M.; Blakeley, R. E.; Mader, D. M.; Hecht, A. A.

    2014-07-09

    A position-sensitive, high-resolution time-of-flight detector for fission fragments has been developed. The SPectrometer for Ion DEtermination in fission Research (SPIDER) is a 2E–2v spectrometer designed to measure the mass of light fission fragments to a single mass unit. The time pick-off detector pairs to be used in SPIDER have been tested with α-particles from 229Th and its decay chain and α-particles and spontaneous fission fragments from 252Cf. Each detector module is comprised of thin electron conversion foil, electrostatic mirror, microchannel plates, and delay-line anodes. Particle trajectories on the order of 700 mm are determined accurately to within 0.7 mm. Flight times were measured with 250 ps resolution FWHM. Computed particle velocities are accurate to within 0.06 mm/ns corresponding to a precision of 0.5%. As a result, an ionization chamber capable of 400 keV energy resolution coupled with the velocity measurements described here will pave the way for modestly efficient measurements of light fission fragments with unit mass resolution.

  17. Development of position-sensitive time-of-flight spectrometer for fission fragment research

    DOE PAGES

    Arnold, C. W.; Tovesson, F.; Meierbachtol, K.; Bredeweg, T.; Jandel, M.; Jorgenson, H. J.; Laptev, A.; Rusev, G.; Shields, D. W.; White, M.; et al

    2014-07-09

    A position-sensitive, high-resolution time-of-flight detector for fission fragments has been developed. The SPectrometer for Ion DEtermination in fission Research (SPIDER) is a 2E–2v spectrometer designed to measure the mass of light fission fragments to a single mass unit. The time pick-off detector pairs to be used in SPIDER have been tested with α-particles from 229Th and its decay chain and α-particles and spontaneous fission fragments from 252Cf. Each detector module is comprised of thin electron conversion foil, electrostatic mirror, microchannel plates, and delay-line anodes. Particle trajectories on the order of 700 mm are determined accurately to within 0.7 mm. Flightmore » times were measured with 250 ps resolution FWHM. Computed particle velocities are accurate to within 0.06 mm/ns corresponding to a precision of 0.5%. As a result, an ionization chamber capable of 400 keV energy resolution coupled with the velocity measurements described here will pave the way for modestly efficient measurements of light fission fragments with unit mass resolution.« less

  18. Total prompt γ-ray emission in fission

    NASA Astrophysics Data System (ADS)

    Wu, C. Y.; Chyzh, A.; Kwan, E.; Henserson, R. A.; Bredeweg, T. A.; Haight, R. C.; Hayes-Sterbenz, A. C.; Lee, H. Y.; O'Donnell, J. M.; Ullmann, J. L.

    2016-06-01

    The total prompt γ-ray energy distributions for the neutron-induced fission of 235U, 239,241Pu at incident neutron energy of 0.025 eV ‒ 100 keV, and the spontaneous fission of 252Cf were measured using the Detector for Advanced Neutron Capture Experiments (DANCE) array in coincidence with the detection of fission fragments by a parallel-plate avalanche counter. DANCE is a highly segmented, highly efficient 4π γ-ray calorimeter. Corrections were made to the measured distribution by unfolding the two-dimension spectrum of total γ-ray energy vs multiplicity using a simulated DANCE response matrix. The mean values of the total prompt γ-ray energy, determined from the unfolded distributions, are ~ 20% higher than those derived from measurements using single γ-ray detector for all the fissile nuclei studied. This raises serious concern on the validity of the mean total prompt γ-ray energy obtained from the product of mean values for both prompt γ-ray energy and multiplicity.

  19. Neutron Capture and Fission Measurements on Actinides at Dance

    NASA Astrophysics Data System (ADS)

    Chyzh, A.; Wu, C. Y.; Kwan, E.; Henderson, R. A.; Gostic, J. M.; Ullmann, J. L.; Bredeweg, T. A.; Jandel, M.; Couture, A. J.; O'Donnell, J. M.; Haight, R. C.; Lee, H. Y.

    2013-03-01

    The prompt γ-ray energy and multiplicity distributions in the spontaneous fission of 252Cf have been measured using a highly granular 4π γ-ray calorimeter. Corrections were made for both energy and multiplicity distributions according to the detector response, which is simulated numerically using a model validated with the γ-ray calibration sources. A comparison of the total γray energy distribution was made between the measurement and a simulation by random sampling of the corrected γ-ray energy and multiplicity distributions through the detector response. A reasonable agreement is achieved between the measurement and simulation, indicating weak correlations between γ-ray energy and multiplicity. Moreover, the increasing agreement with increasing multiplicity manifests the stochastic aspect of the prompt γ decay in spontaneous fission. This calorimeter was designed for the study of neutron capture reactions and an example is given, where the238Pu(n, γ) measurement was carried out in the laboratory environment for the first time.

  20. Multidimensionally constrained relativistic Hartree-Bogoliubov study of spontaneous nuclear fission

    NASA Astrophysics Data System (ADS)

    Zhao, Jie; Lu, Bing-Nan; Nikšić, Tamara; Vretenar, Dario

    2015-12-01

    Background: Recent microscopic studies, based on the theoretical framework of nuclear energy density functionals, have analyzed dynamic (least action) and static (minimum energy) fission paths, and it has been shown that in addition to the important role played by nonaxial and/or octupole collective degrees of freedom, fission paths crucially depend on the approximations adopted in calculating the collective inertia. Purpose: To analyze effects of triaxial and octupole deformations, as well as approximations to the collective inertia, on the symmetric and asymmetric spontaneous fission dynamics, and compare with results of recent studies based on the self-consistent Hartree-Fock-Bogoliubov (HFB) method. Methods: Deformation energy surfaces, collective potentials, and perturbative and nonperturbative cranking collective inertia tensors are calculated using the multidimensionally-constrained relativistic Hartree-Bogoliubov (MDC-RHB) model, with the energy density functionals PC-PK1 and DD-PC1. Pairing correlations are treated in the Bogoliubov approximation using a separable pairing force of finite range. The least-action principle is employed to determine dynamic spontaneous fission paths. Results: The dynamics of spontaneous fission of 264Fm and 250Fm is explored. The fission paths, action integrals, and the corresponding half-lives predicted by the functionals PC-PK1 and DD-PC1 are compared and, in the case of 264Fm, discussed in relation with recent results obtained using the HFB model based on the Skyrme functional SkM* and a density dependent mixed pairing interaction. Conclusions: The inclusion of nonaxial quadrupole and octupole shape degrees of freedom is essential for a quantitative analysis of fission dynamics. The action integrals and, consequently, the half-lives crucially depend on the approximation used to calculate the effective collective inertia along the fission path. The perturbative cranking approach underestimates the effects of structural

  1. Superprolate shape of the spontaneous-fission isomer /sup 240/Am/sup m/

    SciTech Connect

    Pauling, L.

    1980-10-01

    A superprolate structure for nuclei with Aapprox.240 proposed in 1965 on the basis of the polyspheron theory leads to the value 0.66 for the deformation parameter ..beta... This value agrees well with a recently reported experimental value, 0.66 +- 0.04 for the spontaneous-fission isomer /sup 240/Am/sup m/, obtained by Bemis et al. from their measurement of the optical isomer shift. This agreement provides additional support for the proposed superprolate structure.

  2. SOURCES: a code for calculating (alpha,n), spontaneous fission, and delayed neutron sources and spectra.

    PubMed

    Wilson, W B; Perry, R T; Charlton, W S; Parish, T A; Shores, E F

    2005-01-01

    SOURCES is a computer code that determines neutron production rates and spectra from (alpha,n) reactions, spontaneous fission and delayed neutron emission owing to the decay of radionuclides in homogeneous media, interface problems and three-region interface problems. The code is also capable of calculating the neutron production rates due to (alpha,n) reactions induced by a monoenergetic beam of alpha particles incident on a slab of target material. The (alpha,n) spectra are calculated using an assumed isotropic angular distribution in the centre-of-mass system with a library of 107 nuclide decay alpha-particle spectra, 24 sets of measured and/or evaluated (alpha,n) cross sections and product nuclide level branching fractions, and functional alpha particle stopping cross sections for Z < 106. Spontaneous fission sources and spectra are calculated with evaluated half-life, spontaneous fission branching and Watt spectrum parameters for 44 actinides. The delayed neutron spectra are taken from an evaluated library of 105 precursors. The code outputs the magnitude and spectra of the resultant neutron sources. It also provides an analysis of the contributions to that source by each nuclide in the problem. PMID:16381695

  3. Impact of low-energy photons on the characteristics of prompt fission γ -ray spectra

    NASA Astrophysics Data System (ADS)

    Oberstedt, A.; Billnert, R.; Hambsch, F.-J.; Oberstedt, S.

    2015-07-01

    In this paper we report on a new study of prompt γ -rays from the spontaneous fission of 252Cf . Photons were measured in coincidence with fission fragments by employing four different lanthanide halide scintillation detectors. Together with results from a previous work of ours, we determined characteristic parameters with high precision, such as the average γ -ray multiplicity ν¯γ=(8.29 ±0.13 ), the average energy per photon ɛγ=(0.80 ±0.02 ) MeV, and the total γ -ray energy release per fission Eγ ,tot=(6.65 ±0.10 ) MeV. The excellent agreement between the individual results obtained in all six measurements proves the good repeatability of the applied experimental technique. The impact of low-energy photons, i.e., below 500 keV, on prompt fission γ -ray spectra characteristics has been investigated as well by comparing our results with those taken with the DANCE detector system, which appears to suffer from absorption effects in the low-energy region. Correction factors for this effect were estimated, giving results comparable to ours as well as to historical ones. From this we demonstrate that the different techniques of determining the average γ -ray multiplicity, either from a properly measured and normalized spectrum or a measured multiplicity distribution, give equivalent and consistent results.

  4. Uranium and plutonium total half-lives and for the spontaneous fission branch

    SciTech Connect

    Holden, N.E.

    1985-01-01

    The long-lived nuclides of the uranium and plutonium elements are of interest for their use in nuclear reactors, as well as in certain safeguard applications, e.g., alpha counting is often used to determine the amount of material present. The total half-life and the half-life for spontaneous fission are evaluated for these various long-lived nuclides of interest. The various experiments have been reanalyzed and recommended values are presented for /sup 232,233,234/U, /sup 235,236,238/U, and for /sup 236,238,239,240,241,242,244/Pu. These values improve upon preliminary estimates previously presented, in particular with respect to the uncertainties reported. The /sup 234/U half-life of 2.456 +- 0.005 x 10/sup 5/ years impacts directly on the 2200 meters/second fission cross section of /sup 235/U, since earlier measurements used values of 2.47 to 2.5 x 10/sup 5/ years and obtained correspondingly lower cross sections. In a similar manner, the /sup 239/Pu half-life is 1.25% lower than earlier estimates, which results in a 1.25% increase in the 2200 m/s fission cross section for /sup 239/Pu in some earlier cross section measurements. The total half-lives for the uranium nuclides were reviewed some time ago. At that time, the only spontaneous fission value which was evaluated was /sup 238/U. Recently, the uranium and plutonium nuclides were reviewed for both total and fission half-lives. The general procedure followed in this paper has been to review each of the experiments and revise the published values for the latest estimates of the various parameters used by the original authors. For the case of the total half-lives of uranium, only differences from the original work have been discussed. 120 refs., 23 tabs.

  5. Possible production of actinide spontaneous fission activities in damped collisions of /sup 209/Bi+/sup 56/Fe

    SciTech Connect

    Viola, V.E. Jr.; Mignerey, A.C.; Breuer, H.; Wolf, K.L.; Glagola, B.G.; Wilcke, W.W.; Schroeder, W.U.; Huizenga, J.R.; Hilscher, D.; Birkelund, J.R.

    1980-07-01

    Results of recent nuclear reaction studies on the /sup 209/Bi+/sup 56/Fe system are analyzed in order to investigate the cross sections for production of spontaneously fissioning species with 90 < or = Z < or = 100. This reaction is nearly identical to those used as the basis for identification of new elements with Z=104 --107, reported to be spontaneous fission emitters. Evidence is presented which indicates that actinide elements are formed with primary yields of the order of millibarns in strongly damped collisions of 464 MeV /sup 56/Fe with /sup 209/Bi. Although strongly depleted by fission competition, final yields of possible spontaneous fission activities /sup 240en-dash244/Am/sup f/, /sup 234en-dash238/Cf, and /sup 242en-dash246/Fm are calculated to be of the order of nanobarns. These results suggest that the spontaneous fission activities observed in similar reactions may be due at least in part to fission decay of actinide elements rather than elements with Z=104 --107.

  6. Fissible Deposit Characterization at the Former Oak Ridge K-25 Gaseous Diffusion Plant by {sup 252}CF-Source-Driven Measurements

    SciTech Connect

    Hannon, T.F.; Mihalczo, J.T.; Mullens, J.A.; Uckan, T.; Valentine, T.E.; Wyatt, M.S.

    1998-05-01

    largest deposits with the {sup 252}Cf-source-driven transmission (CFSDT) technique, an active neutron interrogation method developed for use at the Oak Ridge Y-12 Plant to identify nuclear weapons components in containers. The active CFSDT measurement technique uses CFSDT time-of-flight measurements of prompt neutrons and gamma rays from an externally introduced {sup 252}Cf source.

  7. Spontaneous fission properties of {sup 252,254}No and {sup 256,258}[104] and the disappearance of the outer fission barrier

    SciTech Connect

    Wild, J.F.; Hulet, E.K.; Lougheed, R.W.; Moody, K.J.; Bandong, B.B.; Dougan, R.J.; Veeck, A.

    1993-09-01

    The mass and total kinetic energy distributions from the spontaneous fission of {sup 252}No, {sup 254}No, {sup 256}[104], and {sup 258}[104] were measured. The results, in combination with earlier measurements for {sup 256}No, {sup 258}No, and {sup 262}No, show a sharp transition from asymmetrical mass division in {sup 256}No to symmetrical division for {sup 258}No and {sup 262}No. On the other hand, all isotopes of element 104, including {sup 260}[104], appear to yield broadly symmetrical mass distributions. The total kinetic energies around 200 MeV for the 104 isotopes indicate that they fission by the low-energy mode of bimodal fission. Recent calculations of static potential energy surfaces including higher-order asymmetric deformations suggest that the outer fission barrier is well below the ground state in energy, which accounts for the observance of the symmetric mass division.

  8. Spontaneous fission properties of sup 258 Fm, sup 259 Md, sup 260 Md, sup 258 No, and sup 260 (104): Bimodal fission

    SciTech Connect

    Hulet, E.K.; Wild, J.F.; Dougan, R.J.; Lougheed, R.W.; Landrum, J.H.; Dougan, A.D.; Baisden, P.A.; Henderson, C.M.; Dupzyk, R.J. ); Hahn, R.L.; and others

    1989-08-01

    We have measured the mass and kinetic-energy distributions from the spontaneous fission of {sup 258}Fm, {sup 258}No, {sup 259}Md, {sup 260}Md, and {sup 260}(104). All are observed to fission with a symmetrical division of mass. The total-kinetic-energy distributions strongly deviated from the Gaussian shape characteristically found in the fission of all other actinides. When the total-kinetic-energy distributions are resolved into two Gaussians, the constituent peaks lie near 200 and 233 MeV. We conclude that both low- and high-energy fission modes occur in four of the five nuclides studied. We call this property bimodal fission.'' Even though both modes are possible in the same nuclide, one generally predominates. We offer an explanation for each mode based on shell structures of the fissioning nucleus and of its fragments. The appearance of both modes of fission in this region of the nuclide chart seems to be a coincidence in that the opportunity to divide into near doubly magic Sn fragments occurs in the same region where the second fission barrier is expected to drop in energy below the ground state of the fissioning nucleus. Appropriate paths on the potential-energy surface of deformation have been found by theorists, but no physical grounds have been advanced that would allow the near equal populations we observe traveling each path. We suggest that this failure to find a reason for somewhat equal branching may be a fundamental flaw of current fission models. Assuming the proposed origins of these modes are correct, we conclude the low-energy, but also mass-symmetrical mode is likely to extend to far heavier nuclei. The high-energy mode will be restricted to a smaller region, a realm of nuclei defined by the proximity of the fragments to the strong neutron and proton shells in {sup 132}Sn.

  9. Quantization in Classical Mechanics and Diffusion Mechanism of Alpha Decay, Cluster Radioactivity, Spontaneous Fission

    SciTech Connect

    Rusov, V. D.; Vlasenko, D. S.; Deliyergiyev, M. A.; Mavrodiev, S. Cht.

    2010-05-04

    Based on the Chetaev generalized theorem the Schredinger equation as the stability condition of trajectories in classical dynamics in the presence of dissipative forces is derived. In the framework of this approach the alternative model for unified description of alpha decay, spontaneous fission, cluster radioactivity and is developed. We show the possibility of the classical (without tunneling) description of radioactive decay of heavy nuclei, when the so called noise-induced transition or, in other words, the stochastic channel of radioactive decay conditioned by the Kramers diffusion mechanism is generated under certain conditions.Using the ENSDF nuclear data, we have found the parametrized solutions of the Kramers equation of the Langevin type by the Alexandrov dynamic auto-regularization method (REGN-Dubna program). These solutions describe with high-accuracy the dependences of half-life (the decay probability) of heavy radioactive nuclei on total kinetic energy of daughter decay products.Verification of the inverse problem solution in the framework of the universal Kramers description of alpha decay, spontaneous fission, cluster radioactivity, which based on the newest experimental data for alpha-decay of even-even superheavy nuclei (Z = 114, 116, 118), shows good coincidence of the experimental and theoretical dependences of half-life on alpha-decay energy.

  10. Quantization in Classical Mechanics and Diffusion Mechanism of Alpha Decay, Proton and Cluster Radioactivity, Spontaneous Fission

    SciTech Connect

    Rusov, V. D.; Vlasenko, D. S.; Deliyergiyev, M. A.; Mavrodiev, S. Cht.

    2010-01-01

    Based on the Chetaev generalized theorem the Schroedinger equation as the stability condition of trajectories in classical dynamics in the presence of dissipative forces is derived. In the framework of this approach the alternative model for unified description of alpha decay, spontaneous fission, cluster and proton radioactivity and is developed. We show the possibility of the classical (without tunneling) description of radioactive decay of heavy nuclei, when the so called noise-induced transition or, in other words, the stochastic channel of radioactive decay conditioned by the Kramers diffusion mechanism is generated under certain conditions.Using the ENSDF nuclear data, we have found the parametrized solutions of the Kramers equation of the Langevin type by the Alexandrov dynamic auto-regularization method (REGN-Dubna program). These solutions describe with high-accuracy the dependences of half-life (the decay probability) of heavy radioactive nuclei on total kinetic energy of daughter decay products.Verification of the inverse problem solution in the framework of the universal Kramers description of alpha decay, spontaneous fission, cluster and proton radioactivity, which based on the newest experimental data for alpha-decay of even-even superheavy nuclei (Z = 114, 116, 118), shows good coincidence of the experimental and theoretical dependences of half-life on alpha-decay energy.

  11. A probe for neutron activation analysis in a drill hole using 252Cf, and a Ge(Li) detector cooled by a melting cryogen

    USGS Publications Warehouse

    Tanner, A.B.; Moxham, R.M.; Senftle, F.E.; Baicker, J.A.

    1972-01-01

    A sonde has been built for high-resolution measurement of natural or neutron-induced gamma rays in boreholes. The sonde is 7.3 cm in diameter and about 2.2 m in length and weighs about 16 kg. The lithium-compensated germanium semiconductor detector is stabilized at -185 to -188??C for as much as ten hours by a cryostatic reservoir containing melting propane. During periods when the sonde is not in use the propane is kept frozen by a gravity-fed trickle of liquid nitrogen from a reservoir temporarily attached to the cryostat section. A 252Cf source, shielded from the detector, may be placed in the bottom section of the sonde for anlysis by measurement of neutron-activation or neutron-capture gamma rays. Stability of the cryostat with changing hydrostatic pressure, absence of vibration, lack of need for power to the cryostat during operation, and freedom of orientation make the method desirable for borehole, undersea, space, and some laboratory applications. ?? 1972.

  12. Lifetimes in neutron-rich fission fragments using the differential recoil distance method

    SciTech Connect

    Kruecken, R.; Chou, W.-T.; Cooper, J. R.; Beausang, C. W.; Barton, C. J.; Caprio, M. A.; Casten, R. F.; Hecht, A. A.; Novak, J. R.; Pietralla, N.

    2001-07-01

    Lifetimes in the neutron-rich nuclei {sup 104}Mo, {sup 110}Ru, and {sup 144}Ba were measured using the differential recoil distance method. The experiment was performed with a {sup 252}Cf fission source inside the New Yale Plunger Device. {gamma} rays were detected by the SPEctrometer for Experiments with Doppler shifts at Yale (SPEEDY) while fission fragments with the appropriate kinematics were detected by an array of photocells.

  13. Light-charged-particle emission in the spontaneous fission of /sup 250/Cf, /sup 256/Fm, and /sup 257/Fm

    SciTech Connect

    Wild, J.F.; Baisden, P.A.; Dougan, R.J.; Hulet, E.K.; Lougheed, R.W.; Landrum, J.H.

    1985-08-01

    We have measured the energy spectra for the emission of long-range ..cap alpha.. particles from the spontaneous fission of /sup 250/Cf, /sup 256/Fm, and /sup 257/Fm, and for tritons and protons from the spontaneous fission of /sup 250/Cf and /sup 256/Fm. We have determined ..cap alpha.., triton, and proton emission probabilities and estimated total light-particle emission probabilities for these nuclides. We compare these and known emission probabilities for five other spontaneously fissioning nuclides with the deformation energy available at scission and show that there is a possible correlation that is consistent with a one-body dissipation mechanism for transferring release energy to particle clusters.

  14. Competition between alpha-decay and spontaneous fission at isotopes of superheavy elements Rf, Db, and Sg

    SciTech Connect

    Anghel, Claudia Ioana; Silisteanu, Andrei Octavian

    2015-12-07

    The most important decay modes for heavy and superheavy nuclei are their α-decay and spontaneous fission. This work investigates the evolution and the competition of these decay modes in long isotopic sequences. The partial half-lives are given by minimal sets of parameters extracted from the fit of experimental data and theoretical results. A summary of the experimental and calculated α-decay and spontaneous fission half-lives of the isotopes of elements Rf, Db, and Sg is presented. Some half-life extrapolations for nuclides not yet known are also obtained.

  15. Multidimensionally-constrained relativistic mean-field study of spontaneous fission: Coupling between shape and pairing degrees of freedom

    NASA Astrophysics Data System (ADS)

    Zhao, Jie; Lu, Bing-Nan; Nikšić, Tamara; Vretenar, Dario; Zhou, Shan-Gui

    2016-04-01

    Background: Studies of fission dynamics, based on nuclear energy density functionals, have shown that the coupling between shape and pairing degrees of freedom has a pronounced effect on the nonperturbative collective inertia and, therefore, on dynamic (least-action) spontaneous fission paths and half-lives. Purpose: The aim is to analyze the effects of particle-number fluctuation degrees of freedom on symmetric and asymmetric spontaneous fission (SF) dynamics, and to compare the findings with the results of recent studies based on the self-consistent Hartree-Fock-Bogoliubov (HFB) method. Methods: Collective potentials and nonperturbative cranking collective inertia tensors are calculated using the multidimensionally-constrained relativistic-mean-field (MDC-RMF) model. Pairing correlations are treated in the BCS approximation using a separable pairing force of finite range. Pairing fluctuations are included as a collective variable using a constraint on particle-number dispersion. Fission paths are determined with the dynamic programming method by minimizing the action in multidimensional collective spaces. Results: The dynamics of spontaneous fission of 264Fm and 250Fm are explored. Fission paths, action integrals, and corresponding half-lives computed in the three-dimensional collective space of shape and pairing coordinates, using the relativistic functional DD-PC1 and a separable pairing force of finite range, are compared with results obtained without pairing fluctuations. Results for 264Fm are also discussed in relation with those recently obtained using the HFB model. Conclusions: The inclusion of pairing correlations in the space of collective coordinates favors axially symmetric shapes along the dynamic path of the fissioning system, amplifies pairing as the path traverses the fission barriers, significantly reduces the action integral, and shortens the

  16. Relative biological efficiency for the induction of various gene mutations in normal and enriched with 10B Tradescantia cells by neutrons from 252Cf source.

    PubMed

    Cebulska-Wasilewska, A; Schneider, K; Kim, J K

    2001-03-01

    The effectiveness of neutrons from a Californium-252 source in the induction of various abnormalities in the Tradescantia clone 4430 stamen hair cells (Trad-SH assay) were studied. A special attention was paid to check whether any enhancement in effects is visible in the cells enriched with boron ions. Inflorescences, normal or pretreated with chemicals containing boron, were irradiated in the air with neutrons from a 252Cf source at KAERI, Taejon, Korea. To estimate the relative biological effectiveness (RBE) of the beam under the study, numbers of Tradescantia inflorescence without chemical pretreatment were irradiated with various doses of X-rays. The ranges of radiation doses used for neutrons were 0-1.0Gy and for X-rays 0-0.5Gy. Following the culturing according to standard procedures screening of gene and lethal mutations in somatic cells of stamen hairs was done in the extended period, between days 7 and 19 after exposures. Maximal RBE values for the induction of pink, colorless and lethal mutations were evaluated from comparison of the slopes in linear parts of the dose response curves obtained after irradiation with X-rays and californium source. The RBE(max) value or the induction of gene mutation was estimated as 7.2 comparing the value 5.6 in the studies reported earlier. The comparison of dose-response curves and its alteration, due to changes in the cells and plants environment during and after irradiation, explains the observed differences. Inflorescence pretreated with borax responded to neutrons differently depending on the biological end points. Although, for the induction of pink mutations no significant difference was observed, though, in the case of cell lethality, pretreated with boron ion plants have shoved a statistically significant increase of the RBE value from 5.5 to 34.7, and in the case of colorless mutations from 1.6 to 5.6.

  17. Spontaneous Fission Modes and Lifetimes of Superheavy Elements in the Nuclear Density Functional Theory

    SciTech Connect

    Staszczak, A,

    2013-01-01

    Background: The reactions with the neutron-rich 48Ca beam and actinide targets resulted in the detection of new superheavy (SH) nuclides with Z=104 118. The unambiguous identification of the new isotopes, however, still poses a problem because their -decay chains terminate by spontaneous fission (SF) before reaching the known region of the nuclear chart. The understanding of the competition between -decay and SF channels in SH nuclei is, therefore, of crucial importance for our ability to map the SH region and to assess its extent.

    Purpose: We perform self-consistent calculations of the competing decay modes of even-even SH isotopes with 108 Z 126 and 148 N 188.

    Methods: We use the state-of-the-art computational framework based on self-consistent symmetry-unrestricted nuclear density functional theory capable of describing the competition between nuclear attraction and electrostatic repulsion. We apply the SkM* Skyrme energy density functional. The collective mass tensor of the fissioning superfluid nucleus is computed by means of the cranking approximation to the adiabatic time-dependent Hartree-Fock-Bogoliubov (HFB) approach. This paper constitutes a systematic self-consistent study of spontaneous fission in the SH region, carried out at a full HFB level, that simultaneously takes into account both triaxiality and reflection asymmetry.

    Results: Breaking axial symmetry and parity turns out to be crucial for a realistic estimate of collective action; it results in lowering SF lifetimes by more than 7 orders of magnitude in some cases. We predict two competing SF modes: reflection symmetric modes and reflection asymmetric modes.

    Conclusions: The shortest-lived SH isotopes decay by SF; they are expected to lie in a narrow corridor formed by 280Hs, 284Fl, and 118284Uuo that separates the regions of SH nuclei synthesized in cold-fusion and hot-fusion reactions. The region of long-lived SH nuclei is expected to be centered on 294Ds with a total half-life of

  18. 1987 Neutron and gamma personnel dosimeter intercomparison study using a D/sub 2/O-moderated /sup 252/Cf source

    SciTech Connect

    Swaja, R.E.; West, L.E.; Sims, C.S.; Welty, T.J.

    1989-05-01

    The thirteenth Personnel Dosimetry Intercomparison Study (i.e., PDIS 13) was conducted during April 1987 as a joint effort by Oak Ridge National Laboratory's (ORNL) Dosimetry Applications Research Group and the Southwest Radiation Calibration Center at the University of Arkansas. A total of 48 organizations (34 from the US and 14 from abroad) participated in PDIS 13. Participants submitted a total of 1,113 neutron and gamma dosimeters for this mixed field study. The dosimeters were transferred by mail and were handled by experimental personnel at ORNL and the University of Arkansas. The type of neutron dosimeter and the percentage of participants submitting that type are as follows: TLD-albedo (49%), direct interaction TLD (31%), CR-39 (17%), film (3%). The type of gamma dosimeter and the percentage of participants submitting that type are as follows: Li/sub 2/B/sub 4/O/sub 7/, alone or in combination with CaSO/sub 4/, (69%), /sup 7/LiF (28%), natural LiF (3%). Radiation exposures in PDIS 13 were limited to 0.5 and 1.5 mSv from /sup 252/Cf moderated by 15-cm of D/sub 2/O. Traditional exposures using the Health Physics Research Reactor (HPRR) were not possible due to the fact that all reactors at ORNL, including the HPRR, were shutdown by order of the Department of Energy at the time the intercomparison was performed. Planned exposures using a /sup 238/PuBe source were negated by a faulty timing mechanism. Based on accuracy and precision, direct interaction TLD dosimeters exhibited the best performance in PDIS 13 neutron measurements. They were followed, in order of best performance, by CR-39, TLD albedo, and film. The Li/sub 2/B/sub 4/O/sub 7/ type TLD dosimeters exhibited the best performance in PDIS 13 gamma measurements. They were followed by natural LiF, /sup 7/LiF, and film. 12 refs., 1 fig., 5 tabs.

  19. Searches for superheavy elements in nature: Cosmic-ray nuclei; spontaneous fission

    NASA Astrophysics Data System (ADS)

    Ter-Akopian, G. M.; Dmitriev, S. N.

    2015-12-01

    There is little chance that superheavy nuclei with lifetimes of no less than 100 million years are present on the stability island discovered at present. Also, pessimistic are the results of estimates made about their nucleosynthesis in r-process. Nevertheless, the search for these nuclei in nature is justified in view of the fundamental importance of this topic. The first statistically significant data set was obtained by the LDEF Ultra-Heavy Cosmic-Ray Experiment, consisting of 35 tracks of actinide nuclei in galactic cosmic rays. Because of their exceptionally long exposure time in Galaxy, olivine crystals extracted from meteorites generate interest as detectors providing unique data regarding the nuclear composition of ancient cosmic rays. The contemporary searches for superheavy elements in the earth matter rely on knowledge obtained from chemical studies of artificially synthesized superheavy nuclei. New results finding out the chemical behavior of superheavy elements should be employed to obtain samples enriched in their homologues. The detection of rare spontaneous fission events and the technique of accelerator mass spectrometry are employed in these experiments.

  20. Americium and curium total half-lives and for the spontaneous fission branch

    SciTech Connect

    Holden, N.E.

    1985-01-01

    The long-lived nuclides of the americium and curium elements are of interest for their use in certain safeguard applications and for nuclear reactor burnup studies in waste management. Recommended values are presented for /sup 241,242m,243/Am, and for /sup 242,243,244,245,246,247,248,250/Cm. These values result from a consistent evaluation of all these half-lives. These preliminary estimates were presented earlier. The uncertainties are provided at the 95% confidence limit for each of the recommended values. It will be noted that many of the recommended errors considerably exceed errors quoted by individual authors in their publication, by up to an order of magnitude, e.g. the total half-life of /sup 242,246,248/Cm and the spontaneous fission half-life of /sup 244/Cm. These preliminary estimates for the half-lives were given previously. Efforts continue to reevaluate the various experiments to better gauge the systematic errors involved and reassess the total error.

  1. Advanced modeling of prompt fission neutrons

    SciTech Connect

    Talou, Patrick

    2009-01-01

    Theoretical and numerical studies of prompt fission neutrons are presented. The main results of the Los Alamos model often used in nuclear data evaluation work are reviewed briefly, and a preliminary assessment of uncertainties associated with the evaluated prompt fission neutron spectrum for n (0.5 MeV)+{sup 239}Pu is discussed. Advanced modeling of prompt fission neutrons is done by Monte Carlo simulations of the evaporation process of the excited primary fission fragments. The successive emissions of neutrons are followed in the statistical formalism framework, and detailed information, beyond average quantities, can be inferred. This approach is applied to the following reactions: {sup 252}Cf (sf), n{sub th} + {sup 239}Pu, n (0.5 MeV)+{sup 235}U, and {sup 236}Pu (sf). A discussion on the merits and present limitations of this approach concludes this presentation.

  2. Observation of new spontaneous fission activities from elements 100 to 105

    SciTech Connect

    Somerville, L.P.

    1982-03-01

    Several new Spontaneous Fission (SF) activities have been found. No definite identification could be made for any of the new SF activities; however, half-lives and possible assignments to element-104 isotopes consistent with several cross bombardments include /sup 257/Rf(3.8 s, 14% SF), /sup 258/Rf(13 ms), /sup 259/Rf(approx. 3 s, 8% SF), /sup 260/Rf(approx. 20 ms), and /sup 262/Rf(approx. 50 ms). The 80-ms SF activity claimed by the Dubna group for the discovery of element 104 (/sup 260/104) was not observed. A difficulty exists in the interpretation that /sup 260/Rf is a approx. 20-ms SF activity: in order to be correct, for example, the SF activities with half-lives between 14 and 24 ms produced in the reactions 109- to 119-MeV /sup 18/O + /sup 248/Cm, 88- to 100-MeV /sup 15/N + /sup 249/Bk, and 96-MeV /sup 18/O + /sup 249/Cf must be other nuclides due to their large production cross sections, or the cross sections for production of /sup 260/Rf must be enhanced by unknown mechanisms. Based on calculated total production cross sections a possible approx. 1% electron-capture branch in /sup 258/Lr(4.5 s) to the SF emitter /sup 258/No(1.2 ms) and an upper limit of 0.05% for SF branching in /sup 254/No(55 s) were determined. Other measured half-lives from unknown nuclides produced in respective reactions include approx. 1.6 s (/sup 18/O + /sup 248/CM), indications of a approx. 47-s SF activity (75-MeV /sup 12/C + /sup 249/Cf), and two or more SF activities with 3 s less than or equal to T/sub 1/2/ less than or equal to 60 s (/sup 18/O + /sup 249/Bk). The most exciting conclusion of this work is that if the tentative assignments to even-even element 104 isotopes are correct, there would be a sudden change in the SF half-life systematics at element 104 which has been predicted theoretically and attributed to the disappearance of the second hump of the double-humped fission barrier.

  3. 12. 3-min /sup 256/Cf and 43-min /sup 258/Md and systematics of the spontaneous fission propertiesof heavy nuclides

    SciTech Connect

    Hoffman, D.C.; Wilhelmy, J.B.; Weber, J.; Daniels, W.R.; Hulet, E.K.; Lougheed, R.W.; Landrum, J.H.; Wild, J.F.; Dupzyk, R.J.

    1980-03-01

    The new isotope 12.3-min /sup 256/Cf was produced via the /sup 254/Cf(t,p) reaction, and a new 43-min isomer of /sup 258/Md was produced via the /sup 255/Es(..cap alpha..,n) reaction. The fragment mass and kinetic energy distributions from the spontaneous fission of /sup 256/Cf were found to be very similar to those from the spontaneous fission of lighter Cf isotopes. The mass division is primarily asymmetric, and the average total kinetic energy is 189.8 +- 0.9 MeV. The 43-min /sup 258/Md presumably decays by electron capture and provides an opportunity to study the mass and kinetic energy distributions from the spontaneous fission of the 380-..mu..s /sup 258/Fm daughter. The observed narrow, symmetric mass distribution and the most probable total kinetic energy of 238 +- 3 MeV are similar to those reported for the spontaneous fission of /sup 259/Fm but show a sharp increase in symmetric mass division and total kinetic energy compared to /sup 257/Fm and the lighter Fm isotopes. No such abrupt change in properties was observed for /sup 256/Cf, which, like /sup 258/Fm, has 158 neutrons. The marked difference between the spontaneous fission properties of the heavier Fm isotopes and those of other spontaneously fissioning nuclides is compared to some theoretical predictions.

  4. Code System for Calculating Alpha, N; Spontaneous Fission; and Delayed Neutron Sources and Spectra.

    2002-07-18

    Version: 04 SOURCES4C is a code system that determines neutron production rates and spectra from (alpha,n) reactions, spontaneous fission, and delayed neutron emission due to radionuclide decay. In this release the three-region problem was modified to correct several bugs, and new documentation was added to the package. Details are available in the included LA-UR-02-1617 (2002) report. The code is capable of calculating (alpha,n) source rates and spectra in four types of problems: homogeneous media (i.e.,more » an intimate mixture of alpha-emitting source material and low-Z target material), two-region interface problems (i.e., a slab of alpha-emitting source material in contact with a slab of low-Z target material), three-region interface problems (i.e., a thin slab of low-Z target material sandwiched between alpha-emitting source material and low-Z target material), and (alpha,n) reactions induced by a monoenergetic beam of alpha-particles incident on a slab of target material. The process of creating a SOURCES input file (tape1) is streamlined with the Los Alamos SOURCES Tape1 Creator and Library Link (LASTCALL) Version 1. Intended to supplement the SOURCES manual, LASTCALL is a simple graphical user interface designed to minimize common errors made during input. The optional application, LASTCALL, consists of a single dialog window launched from an executable (lastcall.exe) on Windows-based personal computers.« less

  5. Quantum and Thermodynamic Properties of Spontaneous and Low-Energy Induced Fission of Nuclei

    SciTech Connect

    Kadmensky, S.G.

    2005-12-01

    It is shown that A. Bohr's concept of transition fission states can be matched with the properties of Coriolis interaction if an axisymmetric fissile nucleus near the scission point remains cold despite a nonadiabatic character of nuclear collective deformation motion. The quantum and thermodynamic properties of various stages of binary and ternary fission after the descent of a fissile nucleus from the outer saddle point are studied within quantum-mechanical fission theory. It is shown that two-particle nucleon-nucleon correlations--in particular, superfluid correlations--play an important role in the formation of fission products and in the classification of fission transitions. The distributions of thermalized primary fission fragments with respect to spins and their projections onto the symmetry axis of the fissile nucleus and fission fragments are constructed, these distributions determining the properties of prompt neutrons and gamma rays emitted by these fragments. A new nonevaporation mechanism of third-particle production in ternary fission is proposed. This mechanism involves transitions of third particles from the cluster states of the fissile-nucleus neck to high-energy states under effects of the shake-off type that are due to the nonadiabatic character of nuclear collective deformation motion.

  6. Benchmarking nuclear fission theory

    DOE PAGES

    Bertsch, G. F.; Loveland, W.; Nazarewicz, W.; Talou, P.

    2015-05-14

    We suggest a small set of fission observables to be used as test cases for validation of theoretical calculations. Thus, the purpose is to provide common data to facilitate the comparison of different fission theories and models. The proposed observables are chosen from fission barriers, spontaneous fission lifetimes, fission yield characteristics, and fission isomer excitation energies.

  7. SOURCES 4A: A Code for Calculating (alpha,n), Spontaneous Fission, and Delayed Neutron Sources and Spectra

    SciTech Connect

    Madland, D.G.; Arthur, E.D.; Estes, G.P.; Stewart, J.E.; Bozoian, M.; Perry, R.T.; Parish, T.A.; Brown, T.H.; England, T.R.; Wilson, W.B.; Charlton, W.S.

    1999-09-01

    SOURCES 4A is a computer code that determines neutron production rates and spectra from ({alpha},n) reactions, spontaneous fission, and delayed neutron emission due to the decay of radionuclides. The code is capable of calculating ({alpha},n) source rates and spectra in four types of problems: homogeneous media (i.e., a mixture of {alpha}-emitting source material and low-Z target material), two-region interface problems (i.e., a slab of {alpha}-emitting source material in contact with a slab of low-Z target material), three-region interface problems (i.e., a thin slab of low-Z target material sandwiched between {alpha}-emitting source material and low-Z target material), and ({alpha},n) reactions induced by a monoenergetic beam of {alpha}-particles incident on a slab of target material. Spontaneous fission spectra are calculated with evaluated half-life, spontaneous fission branching, and Watt spectrum parameters for 43 actinides. The ({alpha},n) spectra are calculated using an assumed isotropic angular distribution in the center-of-mass system with a library of 89 nuclide decay {alpha}-particle spectra, 24 sets of measured and/or evaluated ({alpha},n) cross sections and product nuclide level branching fractions, and functional {alpha}-particle stopping cross sections for Z < 106. The delayed neutron spectra are taken from an evaluated library of 105 precursors. The code outputs the magnitude and spectra of the resultant neutron source. It also provides an analysis of the contributions to that source by each nuclide in the problem.

  8. SOURCES 4C : a code for calculating ([alpha],n), spontaneous fission, and delayed neutron sources and spectra.

    SciTech Connect

    Wilson, W. B.; Perry, R. T.; Shores, E. F.; Charlton, W. S.; Parish, Theodore A.; Estes, G. P.; Brown, T. H.; Arthur, Edward D. ,; Bozoian, Michael; England, T. R.; Madland, D. G.; Stewart, J. E.

    2002-01-01

    SOURCES 4C is a computer code that determines neutron production rates and spectra from ({alpha},n) reactions, spontaneous fission, and delayed neutron emission due to radionuclide decay. The code is capable of calculating ({alpha},n) source rates and spectra in four types of problems: homogeneous media (i.e., an intimate mixture of a-emitting source material and low-Z target material), two-region interface problems (i.e., a slab of {alpha}-emitting source material in contact with a slab of low-Z target material), three-region interface problems (i.e., a thin slab of low-Z target material sandwiched between {alpha}-emitting source material and low-Z target material), and ({alpha},n) reactions induced by a monoenergetic beam of {alpha}-particles incident on a slab of target material. Spontaneous fission spectra are calculated with evaluated half-life, spontaneous fission branching, and Watt spectrum parameters for 44 actinides. The ({alpha},n) spectra are calculated using an assumed isotropic angular distribution in the center-of-mass system with a library of 107 nuclide decay {alpha}-particle spectra, 24 sets of measured and/or evaluated ({alpha},n) cross sections and product nuclide level branching fractions, and functional {alpha}-particle stopping cross sections for Z < 106. The delayed neutron spectra are taken from an evaluated library of 105 precursors. The code provides the magnitude and spectra, if desired, of the resultant neutron source in addition to an analysis of the'contributions by each nuclide in the problem. LASTCALL, a graphical user interface, is included in the code package.

  9. Observation of new spontaneous fission activities from elements 100 to 105

    SciTech Connect

    Somerville, L.P.

    1982-01-01

    Several new Spontaneous Fission (SF) activities have been found. Their half-lives and production cross sections in several reactions have been measured by collecting and transporting recoils at known speed past mica track detectors. No definite identification could be made for any of the new SF activities; however, half-lives and possible assignments to element-104 isotopes consistent with several cross bombardments include /sup 257/Rf(3.8s, 14% SF), /sup 258/Rf(13 ms), /sup 259/Rf(approx.3s, 8% SF), /sup 260/Rf(approx.20 ms), and /sup 262/Rf(approx.50 ms). The 80-ms SF activity claimed by the Dubna group for the discovery of element 104 (/sup 260/104) was not observed. A difficulty exists in the interpretation that /sup 260/Rf is a approx.20-ms SF activity: in order to be correct, for example, the SF activities with half-lives between 14 and 24 ms produced in the reactions 109- to 119-MeV /sup 18/O + /sup 248/Cm, 88- to 100-MeV /sup 15/N + /sup 249/Bk, and 96-MeV /sup 18/O + /sup 249/Cf must be other nuclides due to their large production cross sections, or the cross sections for production of /sup 268/Rf must be enhanced by unknown mechanisms. Based on calculated total production cross sections a possible approx.1% electron-capture branch in /sup 258/Lr(4.5 s) to the SF emitter /sup 258/No(1.2 ms) and an upper limit of 0.05% for SF branching in /sup 254/No(55 s) were determined. Other measured half-lives from unknown nuclides produced in respective reactions include approx. 1.6 s (/sup 18/O + /sup 248/Cm), indications of a approx.47-s SF activity (75-MeV /sup 12/C + /sup 249/Cf), and two or more SF activities with 3 s less than or equal to T/sub (1/2)/ less than or equal to 60 s (/sup 18/O + /sup 249/Bk).

  10. Breaking of Axial and Reflection Symmetries in Spontaneous Fission of Fermium Isotopes

    NASA Astrophysics Data System (ADS)

    Staszczak, A.; Baran, A.; Nazarewicz, W.

    The nuclear fission phenomenon is a magnificent example of a quantal collective motion during which the nucleus evolves in a multidimensional space representing shapes with different geometries. The triaxial degrees of freedom are usually important around the inner fission barrier, and reduce the fission barrier height by several MeV. Beyond the inner barrier, reflection-asymmetric shapes corresponding to asymmetric elongated fragments come into play. We discuss the interplay between different symmetry breaking mechanisms in the case of even-even fermium isotopes using the Skyrme HFB formalism.

  11. BREAKING OF AXIAL AND REFLECTION SYMMETRIES IN SPONTANEOUS FISSION OF FERMIUM ISOTOPES

    SciTech Connect

    Staszczak, A.; Nazarewicz, Witold; Baran, Andrzej K

    2011-01-01

    The nuclear fission phenomenon is a magnificent example of a quantal collective motion during which the nucleus evolves in a multidimensional space representing shapes with different geometries. The triaxial degrees of freedom are usually important around the inner fission barrier, and reduce the fission barrier height by several MeV. Beyond the inner barrier, reflection-asymmetric shapes corresponding to asymmetric elongated fragments come into play. We discuss the interplay between different symmetry breaking mechanisms in the case of even-even fermium isotopes using the Skyrme HFB formalism.

  12. The half-life of lead with respect to spontaneous fission

    SciTech Connect

    Zakharova, V.P.; Zenkevich, V.S.; Funshtein, V.B.

    1995-04-01

    The authors report results of an experiment to measure the half life of lead 208 against fission. The impetus for this work is earlier work in the case of fermium isotopes, where it was found that addition of two neutrons to fermium, producing isotopes which could decay to fragments with near magic numbers, resulted in tremendous decreases in fission lifetimes. The authors had assumed the same effect could be seen in lead 208. This experiment has put a lower bound of 2{times}10{sup 19} yr on this decay in lead 208.

  13. Fragment mass and kinetic-energy distributions from spontaneous fission of the neutron-deficient isotopes, 1. 2-s /sup 246/Fm and 38-s /sup 248/Fm

    SciTech Connect

    Hoffman, D.; Lee, D.; Ghiorso, A.; Nurmia, M.; Aleklett, K.

    1980-10-01

    We have measured the mass and kinetic-energy distributions for fragments from the spontaneous fission of 1.2-s /sup 246/Fm and 38-s /sup 248/Fm. The mass distributions are highly asymmetric and the average total kinetic energies of 199 +- 4 MeV and 198 +- 4 MeV, respectively, are consistent with systematics for lower Z actinides. Their properties are in contrast to those of /sup 258/Fm and /sup 259/Fm, whose spontaneous fission results in narrowly symmetric mass distributions accompanied by unusually high total kinetic energies.

  14. HALF-LIVES OF LONG-LIVED A-DECAY, B-DECAY, BB-DECAY AND SPONTANEOUS FISSION NUCLIDES.

    SciTech Connect

    HOLDEN,N.E.

    2001-06-29

    In his review of radionuclides for dating purposes, Roth noted that there were a large number of nuclides, normally considered ''stable'' but which are radioactive with a very long half-life. Roth suggested that I review the data on the half-life values of these long-lived nuclides for a discussion session at the next meeting. These half-life values for long-lived nuclides include those due to various decay modes, {alpha}-decay, {beta}-decay, electron capture decay, {beta}{beta}-decay and spontaneous fission decay. This report is preliminary but will provide a quick overview of the extensive table of data on the recommendations from that review.

  15. Prompt Fission γ-ray Spectra Characteristics - A First Summary

    NASA Astrophysics Data System (ADS)

    Oberstedt, S.; Billnert, R.; Gatera, A.; Geerts, W.; Halipré, P.; Hambsch, F.-J.; Lebois, M.; Oberstedt, A.; Marini, P.; Vidali, M.; Wilson, J. N.

    In this work we give an overview of our investigations of prompt γ-ray emission in nuclear fission. This work was conducted during the last five years in response to a high priority nuclear data request formulated by the OECD/NEA. The aim was to reveal data deficiencies responsible for a severe under-prediction of the prompt γ heating in nuclear reactor cores. We obtained new prompt fission γ-ray spectral (PFGS) data for 252Cf(SF) as well as for thermal-neutron induced fission on 235U(nth,f) and 241Pu(nth,f). In addition, first PFGS measurements with a fast-neutron beam were accomplished, too. The impact of the new data and future data needs are discussed.

  16. Sputtering yield of Pu bombarded by fission Fragments from Cf

    SciTech Connect

    Danagoulian, Areg; Klein, Andreas; Mcneil, Wendy V; Yuan, Vincent W

    2008-01-01

    We present results on the yield of sputtering of Pu atoms from a Pu foil, bombarded by fission fragments from a {sup 252}Cf source in transmission geometry. We have found the number of Pu atoms/incoming fission fragments ejected to be 63 {+-} 1. In addition, we show measurements of the sputtering yield as a function of distance from the central axis, which can be understood as an angular distribution of the yield. The results are quite surprising in light of the fact that the Pu foil is several times the thickness of the range of fission fragment particles in Pu. This indicates that models like the binary collision model are not sufficient to explain this behavior.

  17. Isotopic yield in cold binary fission of even-even 244-258Cf isotopes

    NASA Astrophysics Data System (ADS)

    Santhosh, K. P.; Cyriac, Annu; Krishnan, Sreejith

    2016-05-01

    The cold binary fission of even-even 244-258Cf isotopes has been studied by taking the interacting barrier as the sum of Coulomb and proximity potential. The favorable fragment combinations are obtained from the cold valley plot (plot of driving potential vs. mass number of fragments) and by calculating the yield for charge minimized fragments. It is found that for 244,246,248Cf isotopes highest yield is for the fragments with isotope of Pb (Z = 82) as one fragment, whereas for 250Cf and 252Cf isotopes the highest yield is for the fragments with isotope of Hg (Z = 80) as one fragment. In the case of 254,256,258Cf isotopes the highest yield is for the fragments with Sn (Z = 50) as one fragment. Thus, the fragment combinations with maximum yield reveal the role of doubly magic and near doubly magic nuclei in binary fission. It is found that asymmetric splitting is favored for Cf isotopes with mass number A ≤ 250 and symmetric splitting is favored for Cf isotopes with A > 252. In the case of Cf isotope with A = 252, there is an equal probability for asymmetric and symmetric splitting. The individual yields obtained for the cold fission of 252Cf isotope are compared with the experimental data taken from the γ- γ- γ coincidences technique using Gammasphere.

  18. Estimation of 240Pu Mass in a Waste Tank Using Ultra-Sensitive Detection of Radioactive Xenon Isotopes from Spontaneous Fission

    SciTech Connect

    Bowyer, Ted W.; Gesh, Christopher J.; Haas, Derek A.; Hayes, James C.; Mahoney, Lenna A.; Meacham, Joseph E.; Mendoza, Donaldo P.; Olsen, Khris B.; Prinke, Amanda M.; Reid, Bruce D.; Woods, Vincent T.

    2014-12-01

    We report on a technique to detect and quantify the amount of 240Pu in a large tank used to store nuclear waste from plutonium production at the Hanford nuclear site. While the contents of this waste tank are known from previous grab sample measurements, our technique could allow for determination of the amount of 240Pu in the tank without costly sample retrieval and analysis of this highly radioactive material. This technique makes an assumption, which was confirmed, that 240Pu dominates the spontaneous fissions occurring in the tank.

  19. Spontaneous fission of light californium isotopes produced in 206,207,208Pb + 34,36S reactions; new nuclide 238Cf

    NASA Astrophysics Data System (ADS)

    Lazarev, Yu. A.; Shirokovsky, I. V.; Utyonkov, V. K.; Tretyakova, S. P.; Kutner, V. B.

    1995-02-01

    In bombardments of 206,207,208Pb with 34S and 206Pb with 36S, we identified a new spontaneously fissioning isotope 238Cf with T sf ≈ T {1}/{2} = 21 ± 2 ms and obtained evidence of the production of a new isotope 237Cf with T {1}/{2} = 2.1 ± 0.3 s. The spontaneous-fission (SF) decay mode was established for 240Cf; its SF branch was estimated to be bsf ˜ 2 × 10 -2. We measured also bsf ⩽ 1.4 × 10 -4 for 242Cf and estimated bsf ˜ 10 -1 for 237Cf. The production cross sections of 238Cf in the 206,207,208Pb + 34S reactions were measured to be in the range of 0.3 to 1.1 nb. Finally, we probed the influence of the neutron excess in the N = 20 projectile 36S on cross sections of fusion-evaporation reactions occurring on lead targets.

  20. HALF-LIVES OF LONG-LIVED ALPHA DECAY, BETA DECAY, ELECTRON CAPTURE DECAY, BETA BETA-DECAY, PROTON DECAY AND SPONTANEOUS FISSION DECAY NUCLIDES.

    SciTech Connect

    HOLDEN, H.E.

    2003-08-08

    In his review of radionuclides for dating purposes, Roth noted that there were a large number of nuclides, normally considered ''stable'' but which are radioactive with a very long half-life. Roth suggested that I review the data on the half-life values of these long-lived nuclides for the 2001 Atomic Weights Commission meeting in Brisbane. I provided a report, BNL-NCS-68377, to fulfill Roth's request. Peiser has now made a similar suggestion that I review these data for our next Commission meeting in Ottawa for their possible inclusion in our Tables. These half-life values for long-lived nuclides include those due to various decay modes, {alpha}-decay, {beta}-decay, electron capture decay, {beta}{beta}-decay, proton decay and spontaneous fission decay. This data review (post Brisbane) provides an update to the recommendation of the 2001 review.

  1. Neutron production from (. cap alpha. ,n) reactions and spontaneous fission in ThO/sub 2/, UO/sub 2/, and (U,Pu)O/sub 2/ fuels

    SciTech Connect

    Perry, R.T.; Wilson, W.B.

    1981-06-01

    Available alpha-particle stopping cross-section and /sup 17/ /sup 18/O(..cap alpha..,n) cross-section data were adjusted, fitted, and used in calculating the thick-target neutron production function for alpha particles below 10 MeV in oxide fuels. The spent UO/sub 2/ function produced was folded with actinide decay spectra to determine (..cap alpha..,n) neutron production by each of 89 actinides. Spontaneous-fission (SF) neutron production for 40 actinides was calculated as the product of anti ..nu..(SF) and SF branching-fraction values accumulated or estimated from available data. These contributions and total neutron production in spent UO/sub 2/ fuel are tabulated and, when combined with any calculated inventory, describe the spent UO/sub 2/ neutron source. All data are tabulated and methodology is described to permit easy extension to specialized problems.

  2. Fission Fragment Yield, Cross Section and Prompt Neutron and Gamma Emission Data from Actinide Isotopes

    NASA Astrophysics Data System (ADS)

    Hambsch, F.-J.; Oberstedt, S.; Al-Adili, A.; Brys, T.; Billnert, R.; Matei, C.; Oberstedt, A.; Salvador-Castiñeira, P.; Tudora, A.; Vidali, M.

    2014-05-01

    Recent experimental investigations on major and minor actinides at the JRC-IRMM are presented. Fission-fragment distributions of isotopes with vibrational resonances in the sub-threshold fission cross section, i. e. 234,238U, have been measured. For 234U, the impact of an increased neutron multiplicity for the heavy fragments with higher incident neutron energies has been studied as observed in experiment and also recently theoretically predicted. The impact is found to be noticeable on post-neutron mass yields, which are the relevant quantities for a-priori waste assessments. The fission cross sections for 240,242Pu at threshold and in the plateau region are being investigated within the ANDES project. The results show some discrepancies to the ENDF/B-VII.1 evaluation mainly for 242Pu around 1 MeV, where the evaluation exhibits a resonance-like structure not observed so clearly in the present work. The requested target accuracy in design studies of innovative reactor concepts like Gen-IV is in the range of a few percent. In order to be able to respond to requests for measurements of prompt neutron and γ-ray emission in fission JRC-IRMM has also invested in setting up a neutron and γ-ray detector array. The neutron array is called SCINTIA and has so far been tested with 252Cf(SF). For γ-ray multiplicity and spectrum measurements of 252Cf(SF) and 235U(nth, f) lanthanum- and cerium-halide detectors were successfully used.

  3. Theoretical study of the almost sequential mechanism of true ternary fission

    NASA Astrophysics Data System (ADS)

    Tashkhodjaev, R. B.; Muminov, A. I.; Nasirov, A. K.; von Oertzen, W.; Oh, Yongseok

    2015-05-01

    We consider the collinear ternary fission which is a sequential ternary decay with a very short time between the ruptures of two necks connecting the middle cluster of the ternary nuclear system and outer fragments. In particular, we consider the case where the Coulomb field of the first massive fragment separated during the first step of the fission produces a lower pre-scission barrier in the second step of the residual part of the ternary system. In this case, we obtain a probability of about 10-3 per binary fission for the yield of massive clusters such as 70Ni,Ge-8280,86Se, and 94Kr in the ternary fission of 252Cf. These products appear together with the clusters having mass numbers of A =132 -140 . The results show that the yield of a heavy cluster such as Ni-7068 would be followed by a product of A =138 -148 with a large probability as observed in the experimental data obtained with the FOBOS spectrometer at the Joint Institute for Nuclear Research. The third product is not observed. The landscape of the potential-energy surface shows that the configuration of the Ni +Ca +Sn decay channel is lower by about 12 MeV than that of the Ca +Ni +Sn channel. This leads to the fact that the yield of Ni and Sn is large. The analysis on the dependence of the velocity of the middle fragment on mass numbers of the outer products leads to the conclusion that, in the collinear tripartition channel of 252Cf, the middle cluster has a very small velocity, which does not allow it to be found in experiments.

  4. Comparative study of the fragments' mass and energy characteristics in the spontaneous fussion of 238Pu, 240Pu and 242Pu and in the thermal-neutron-induced fission of 239Pu

    NASA Astrophysics Data System (ADS)

    Schillebeeckx, P.; Wagemans, C.; Deruytter, A. J.; Barthélémy, R.

    1992-08-01

    The energy and mass distribution and their correlations have been studied for the spontaneous fission of 238, 240, 242Pu and for the thermal-neutron-induced fission of 239Pu. A comparison of 240Pu(s.f.) and 239Pu(nth,f) shows that the increase in excitation energy mainly results in an increase of the intrinsic excitation energy. A comparison of the results for 238Pu, 240Pu and 242Pu(s.f.) demonstrates the occurence of different fission modes with varying relative probability. These results are discussed in terms of the scission point model as well as in terms of the fission channel model with random neck-rupture.

  5. Bimodal fission

    SciTech Connect

    Hulet, E.K.

    1989-04-19

    In recent years, we have measured the mass and kinetic-energy distributions from the spontaneous fission of /sup 258/Fm, /sup 259/Md, /sup 260/Md, /sup 258/No, /sup 262/No, and /sup 260/(104). All are observed to fission with a symmetrical division of mass, whereas the total-kinetic-energy (TKE) distributions strongly deviated from the Gaussian shape characteristically found in the fission of all other actinides. When the TKE distributions are resolved into two Gaussians the constituent peaks lie near 200 and near 233 MeV. We conclude two modes or bimodal fission is occurring in five of the six nuclides studied. Both modes are possible in the same nuclides, but one generally predominates. We also conclude the low-energy but mass-symmetrical mode is likely to extend to far heavier nuclei; while the high-energy mode will be restricted to a smaller region, a region of nuclei defined by the proximity of the fragments to the strong neutron and proton shells in /sup 132/Sn. 16 refs., 7 figs., 1 tab.

  6. Xe-135 Production from Cf-252

    SciTech Connect

    C. A. McGrath; T. P. Houghton; J. K. Pfeiffer; R. K. Hague

    2012-03-01

    135Xe is a good indicator that fission has occurred and is a valuable isotope that helps enforce the Comprehensive Test Ban Treaty. Due to its rather short half life and minimal commercial interest, there are no known sources where 135Xe can be purchased. Readily available standards of this isotope for calibrating collection and analytical techniques would be very useful. 135Xe can be produced in the fissioning of actinide isotopes, or by neutron capture on 134Xe. Since the neutron capture cross section of 134Xe is 3 mB, neutron capture is a low yield, though potentially useful, production route. 135Xe is also produced by spontaneous fission of 252Cf. 252Cf has a spontaneous fission rate of about 6 x 1011 s-1g-1. The cumulative yield from the spontaneous fission of 252Cf is 4.19%; and the competing neutron capture reaction that depletes 135Xe in thermal reactor systems is negligible because the neutron capture cross-section is low for fast fission neutrons. At the INL, scientists have previously transported fission products from an electroplated 252Cf thin source for the measurement of nuclear data of short-lived fission products using a technique called He-Jet collection. We have applied a similar system to the collection of gaseous 135Xe, in order to produce valuable standards of this isotope.

  7. Monte-Carlo Hauser-Feshbach simulations of prompt fission gamma-ray properties

    NASA Astrophysics Data System (ADS)

    Stetcu, Ionel; Talou, Patrick; Kawano, Toshihiko; Jandel, Marian

    2014-09-01

    Properties of prompt fission neutrons and γ rays, emitted before the weak decays of the fission fragments toward stability, are important for both nuclear technologies and a better understanding of the fission process. In the present work, we use the Hauser-Feshbach model to simulate the de-excitation of the fully accelerated fission fragments treated as compound nuclei. Our Monte-Carlo implementation of the Hauser-Feshbach statistical model, which takes into account the competition between the neutron and γ emissions, allows the description of both average quantities, like in the Los Alamos model, and correlations between the emitted particles. Our simulations will be compared against available experimental data and current evaluations. In particular, we will compare our average γ-ray spectrum with recent measurements at the research reactor KFKI in Budapest for the 235U(nth , f) and 252Cf(sf) reactions, as well as multiplicity-dependent distributions obtained at the DANCE facility at LANSCE. Properties of prompt fission neutrons and γ rays, emitted before the weak decays of the fission fragments toward stability, are important for both nuclear technologies and a better understanding of the fission process. In the present work, we use the Hauser-Feshbach model to simulate the de-excitation of the fully accelerated fission fragments treated as compound nuclei. Our Monte-Carlo implementation of the Hauser-Feshbach statistical model, which takes into account the competition between the neutron and γ emissions, allows the description of both average quantities, like in the Los Alamos model, and correlations between the emitted particles. Our simulations will be compared against available experimental data and current evaluations. In particular, we will compare our average γ-ray spectrum with recent measurements at the research reactor KFKI in Budapest for the 235U(nth , f) and 252Cf(sf) reactions, as well as multiplicity-dependent distributions obtained at the

  8. Thermal fission rates with temperature dependent fission barriers

    NASA Astrophysics Data System (ADS)

    Zhu, Yi; Pei, J. C.

    2016-08-01

    Background: The fission processes of thermal excited nuclei are conventionally studied by statistical models which rely on inputs of phenomenological level densities and potential barriers. Therefore the microscopic descriptions of spontaneous fission and induced fission are very desirable for a unified understanding of various fission processes. Purpose: We propose to study the fission rates, at both low and high temperatures, with microscopically calculated temperature-dependent fission barriers and collective mass parameters. Methods: The fission barriers are calculated by the finite-temperature Skyrme-Hartree-Fock+BCS method. The mass parameters are calculated by the temperature-dependent cranking approximation. The thermal fission rates can be obtained by the imaginary free energy approach at all temperatures, in which fission barriers are naturally temperature dependent. The fission at low temperatures can be described mainly as a barrier-tunneling process. While the fission at high temperatures has to incorporate the reflection above barriers. Results: Our results of spontaneous fission rates reasonably agree with other studies and experiments. The temperature dependencies of fission barrier heights and curvatures have been discussed. The temperature dependent behaviors of mass parameters have also been discussed. The thermal fission rates from low to high temperatures with a smooth connection have been given by different approaches. Conclusions: Since the temperature dependencies of fission barrier heights and curvatures, and the mass parameters can vary rapidly for different nuclei, the microscopic descriptions of thermal fission rates are very valuable. Our studies without free parameters provide a consistent picture to study various fissions such as that in fast-neutron reactors, astrophysical environments, and fusion reactions for superheavy nuclei.

  9. Benchmark test of neutron transport calculations: indium, nickel, gold, europium, and cobalt activation with and without energy moderated fission neutrons by iron simulating the Hiroshima atomic bomb casing.

    PubMed

    Iwatani, K; Hoshi, M; Shizuma, K; Hiraoka, M; Hayakawa, N; Oka, T; Hasai, H

    1994-10-01

    A benchmark test of the Monte Carlo neutron and photon transport code system (MCNP) was performed using a bare- and energy-moderated 252Cf fission neutron source which was obtained by transmission through 10-cm-thick iron. An iron plate was used to simulate the effect of the Hiroshima atomic bomb casing. This test includes the activation of indium and nickel for fast neutrons and gold, europium, and cobalt for thermal and epithermal neutrons, which were inserted in the moderators. The latter two activations are also to validate 152Eu and 60Co activity data obtained from the atomic bomb-exposed specimens collected at Hiroshima and Nagasaki, Japan. The neutron moderators used were Lucite and Nylon 6 and the total thickness of each moderator was 60 cm or 65 cm. Measured activity data (reaction yield) of the neutron-irradiated detectors in these moderators decreased to about 1/1,000th or 1/10,000th, which corresponds to about 1,500 m ground distance from the hypocenter in Hiroshima. For all of the indium, nickel, and gold activity data, the measured and calculated values agreed within 25%, and the corresponding values for europium and cobalt were within 40%. From this study, the MCNP code was found to be accurate enough for the bare- and energy-moderated 252Cf neutron activation calculations of these elements using moderators containing hydrogen, carbon, nitrogen, and oxygen. PMID:8083048

  10. Benchmark test of neutron transport calculations: Indium, nickel, gold, europium, and cobalt activation with and without energy moderated fission neutrons by iron simulating the Hiroshima atomic bomb casing

    SciTech Connect

    Iwatani, Kazuo; Shizuma, Kiyoshi; Hasai, Hiromi; Hoshi, Masaharu; Hiraoka, Masayuki; Hayakawa, Norihiko; Oka, Takamitsu

    1994-10-01

    A benchmark test of the Monte Carlo neutron and photon transport code system (MCNP) was performed using a bare- and energy-moderated {sup 252}Cf fission neutron source which was obtained by transmission through 10-cm-thick iron. An iron plate was used to simulate the effect of the Hiroshima atomic bomb casing. This test includes the activation of indium and nickel for fast neutrons and gold, europium, and cobalt for thermal and epithermal neutrons, which were inserted in the moderators. The latter two activations are also to validate {sup 152}Eu and {sup 60}Co activity data obtained from the atomic bomb-exposed specimens collected at Hiroshima and Nagasaki, Japan. The neutron moderators used were Lucite and Nylon 6 and the total thickness of each moderator was 60 cm or 65 cm. Measured activity data (reaction yield) of the neutron-irradiated detectors in these moderators decreased to about 1/1,000th or 1/10,000th, which corresponds to about 1,500 m ground distance from the hypocenter in Hiroshima. For all of the indium, nickel, and gold activity data, the measured and calculated values agreed within 25%, and the corresponding values for europium and cobalt were within 40%. From this study, the MCNP code was found to be accurate enough for the bare- and energy-moderated {sup 252}Cf neutron activation calculations of these elements using moderators containing hydrogen, carbon, nitrogen, and oxygen. 18 refs., 10 figs., 4 tabs.

  11. Benchmark test of neutron transport calculations: indium, nickel, gold, europium, and cobalt activation with and without energy moderated fission neutrons by iron simulating the Hiroshima atomic bomb casing.

    PubMed

    Iwatani, K; Hoshi, M; Shizuma, K; Hiraoka, M; Hayakawa, N; Oka, T; Hasai, H

    1994-10-01

    A benchmark test of the Monte Carlo neutron and photon transport code system (MCNP) was performed using a bare- and energy-moderated 252Cf fission neutron source which was obtained by transmission through 10-cm-thick iron. An iron plate was used to simulate the effect of the Hiroshima atomic bomb casing. This test includes the activation of indium and nickel for fast neutrons and gold, europium, and cobalt for thermal and epithermal neutrons, which were inserted in the moderators. The latter two activations are also to validate 152Eu and 60Co activity data obtained from the atomic bomb-exposed specimens collected at Hiroshima and Nagasaki, Japan. The neutron moderators used were Lucite and Nylon 6 and the total thickness of each moderator was 60 cm or 65 cm. Measured activity data (reaction yield) of the neutron-irradiated detectors in these moderators decreased to about 1/1,000th or 1/10,000th, which corresponds to about 1,500 m ground distance from the hypocenter in Hiroshima. For all of the indium, nickel, and gold activity data, the measured and calculated values agreed within 25%, and the corresponding values for europium and cobalt were within 40%. From this study, the MCNP code was found to be accurate enough for the bare- and energy-moderated 252Cf neutron activation calculations of these elements using moderators containing hydrogen, carbon, nitrogen, and oxygen.

  12. Radioactive beams from Californium fission at the CARIBU facility

    NASA Astrophysics Data System (ADS)

    Savard, Guy; Pardo, Richard; Baker, Sam; Davids, Cary; Peterson, Don; Phillips, Don; Vondrasek, Rick; Zabransky, Bruce; Zinkann, Gary

    2009-10-01

    The Californium Rare Ion Breeder Upgrade (CARIBU) of the ATLAS superconducting linac facility aims at providing low energy and reaccelerated neutron-rich radioactive beams to address key nuclear physics and astrophysics questions. These beams are obtained from fission fragments of a 1 Ci ^252Cf source, thermalized and collected into a low-energy particle beam by a helium gas catcher, mass analyzed by an isobar separator, and charge breed to higher charge states for acceleration in ATLAS. The method described is fast and universal and short-lived isotope yield scale essentially with Californium fission yields. Expected intensities of reaccelerated beams are up to ˜5x10^5 (10^7 at low energy) far-from-stability ions per second on target. Initial commissioning is being performed with weaker 2.5 and 80 mCi sources. Commissioning results, together with the nuclear physics and astrophysics program that will be pursued with the neutron-rich beams made available, will be presented. Plans for installation of the 1 Ci source will be discussed.

  13. Fission fragment mass and energy distributions as a function of incident neutron energy measured in a lead slowing-down spectrometer

    SciTech Connect

    Romano, C.; Danon, Y.; Block, R.; Thompson, J.; Blain, E.; Bond, E.

    2010-01-15

    A new method of measuring fission fragment mass and energy distributions as a function of incident neutron energy in the range from below 0.1 eV to 1 keV has been developed. The method involves placing a double-sided Frisch-gridded fission chamber in Rensselaer Polytechnic Institute's lead slowing-down spectrometer (LSDS). The high neutron flux of the LSDS allows for the measurement of the energy-dependent, neutron-induced fission cross sections simultaneously with the mass and kinetic energy of the fission fragments of various small samples. The samples may be isotopes that are not available in large quantities (submicrograms) or with small fission cross sections (microbarns). The fission chamber consists of two anodes shielded by Frisch grids on either side of a single cathode. The sample is located in the center of the cathode and is made by depositing small amounts of actinides on very thin films. The chamber was successfully tested and calibrated using 0.41+-0.04 ng of {sup 252}Cf and the resulting mass distributions were compared to those of previous work. As a proof of concept, the chamber was placed in the LSDS to measure the neutron-induced fission cross section and fragment mass and energy distributions of 25.3+-0.5 mug of {sup 235}U. Changes in the mass distributions as a function of incident neutron energy are evident and are examined using the multimodal fission mode model.

  14. Microscopic description of complex nuclear decay: Multimodal fission

    NASA Astrophysics Data System (ADS)

    Staszczak, A.; Baran, A.; Dobaczewski, J.; Nazarewicz, W.

    2009-07-01

    Our understanding of nuclear fission, a fundamental nuclear decay, is still incomplete due to the complexity of the process. In this paper, we describe a study of spontaneous fission using the symmetry-unrestricted nuclear density functional theory. Our results show that the observed bimodal fission can be explained in terms of pathways in multidimensional collective space corresponding to different geometries of fission products. We also predict a new phenomenon of trimodal spontaneous fission for some rutherfordium, seaborgium, and hassium isotopes.

  15. Microscopic description of complex nuclear decay: Multimodal fission

    SciTech Connect

    Staszczak, A.; Baran, A.; Dobaczewski, J.; Nazarewicz, W.

    2009-07-15

    Our understanding of nuclear fission, a fundamental nuclear decay, is still incomplete due to the complexity of the process. In this paper, we describe a study of spontaneous fission using the symmetry-unrestricted nuclear density functional theory. Our results show that the observed bimodal fission can be explained in terms of pathways in multidimensional collective space corresponding to different geometries of fission products. We also predict a new phenomenon of trimodal spontaneous fission for some rutherfordium, seaborgium, and hassium isotopes.

  16. Microstructure damage of thin aluminum films by irradiation with alpha particles and fission fragments

    SciTech Connect

    Sadi, S.; Paulenova, A.; Loveland, W.D.; Watson, P.R.

    2007-07-01

    The atomic force microscopy (AFM) has been used to study the microstructure damage of thin aluminum film surfaces induced by bombardment of alpha particles and fission fragments from {sup 252}Cf source. Different types of defects (dislocations lines, loops, voids, and blisters) and their complex morphologies appeared under both the beam of alpha particles and a mix of alpha particles and fission fragments. The first surface damage became clearly visible only after 250 hr irradiation of a mix of alpha particles and fission fragments (8.65 x 10{sup 8} ff/cm{sup 2} and 1.36 x 10{sup 10} {alpha}/cm{sup 2}). The number of voids and dislocation lines created on the aluminum surface were (3.8 {+-} 0.8) x 10{sup 7} cm{sup -2} and (2.1 {+-} 0.8) x 10{sup 6} cm{sup -2}, respectively. Single blisters were observed with the mean diameter of (933 {+-} 22) nm and the mean height of (102 {+-} 15) nm. The first ellipsoidal dislocation loops appeared at the fluence of (1.03 x 10{sup 9} ff/cm{sup 2} and 1.62 x 10{sup 10} {alpha}/cm{sup 2}). However, these ellipsoidal loops were not seen with low energetic alpha particles at the same fluence. Our results suggest that the fission fragments might maximize large voids and dislocations and increase the degradation in depth resolution. (authors)

  17. Fission Particle Emission Multiplicity Simulation

    2006-09-27

    Simulates discrete neutron and gamma-ray emission from the fission of heavy nuclei that is either spontaneous or neutron induced. This is a function library that encapsulates the fission physics and is intended to be called Monte Carlo transport code.

  18. Investigation of phenomenological models for the Monte Carlo simulation of the prompt fission neutron and {gamma} emission

    SciTech Connect

    Litaize, O.; Serot, O.

    2010-11-15

    A Monte Carlo simulation of the fission fragment deexcitation process was developed in order to analyze and predict postfission-related nuclear data which are of crucial importance for basic and applied nuclear physics. The basic ideas of such a simulation were already developed in the past. In the present work, a refined model is proposed in order to make a reliable description of the distributions related to fission fragments as well as to prompt neutron and {gamma} energies and multiplicities. This refined model is mainly based on a mass-dependent temperature ratio law used for the initial excitation energy partition of the fission fragments and a spin-dependent excitation energy limit for neutron emission. These phenomenological improvements allow us to reproduce with a good agreement the {sup 252}Cf(sf) experimental data on prompt fission neutron multiplicity {nu}(A), {nu}(TKE), the neutron multiplicity distribution P({nu}), as well as their energy spectra N(E), and lastly the energy release in fission.

  19. The SPIDER fission fragment spectrometer for fission product yield measurements

    SciTech Connect

    Meierbachtol, K.; Tovesson, F.; Shields, D.; Arnold, C.; Blakeley, R.; Bredeweg, T.; Devlin, M.; Hecht, A. A.; Heffern, L. E.; Jorgenson, J.; Laptev, A.; Mader, D.; O׳Donnell, J. M.; Sierk, A.; White, M.

    2015-04-01

    The SPectrometer for Ion DEtermination in fission Research (SPIDER) developed for measuring mass yield distributions of fission products from spontaneous and neutron-induced fission. The 2E–2v method of measuring the kinetic energy (E) and velocity (v) of both outgoing fission products utilized, with the goal of measuring the mass of the fission products with an average resolution of 1 atomic mass unit (amu). The SPIDER instrument, consisting of detector components for time-of-flight, trajectory, and energy measurements, assembled and tested using 229Th and 252Cf radioactive decay sources. For commissioning, the fully assembled system measured fission products from spontaneous fission of 252Cf. Finally, individual measurement resolutions were met for time-of-flight (250 ps FWHM), spacial resolution (2 mm FHWM), and energy (92 keV FWHM for 8.376 MeV). These mass yield results measured from 252Cf spontaneous fission products are reported from an E–v measurement.

  20. Simultaneous measurement of (n,γ) and (n,fission) cross sections with the DANCE array

    NASA Astrophysics Data System (ADS)

    Bredeweg, T. A.; Jandel, M.; Fowler, M. M.; Bond, E. M.; O'Donnell, J. M.; Reifarth, R.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Wouters, J. M.; Macri, R. A.; Wu, C. Y.; Becker, J. A.

    2006-10-01

    We have recently begun a program of high precision measurements of the key production and destruction reactions of important radiochemical diagnostic isotopes, including several isotopes of uranium, plutonium and americium. The Detector for Advanced Neutron Capture Experiments (DANCE), a 4π BaF2 array located at the Los Alamos Neutron Science Center, will be used to measure the neutron capture cross sections for most of the isotopes of interest. Since neutron capture measurements on many of the actinides are complicated by the presence of γ-rays arising from low-energy neutron-induced fission, we are currently using a dual parallel-plate avalanche counter with the target material electro-deposited directly on the center cathode foil. This design provides a high efficiency for detecting fission fragments and allows loading of pre-assembled target/detector assemblies into the neutron beam line at DANCE. An outline of the current experimental program will be presented as well as results from measurements on ^235U and ^252Cf that utilized the fission-tag detector.

  1. Simultaneous measurement of (n, γ) and (n, fission) cross sections with the DANCE 4π BaF 2 array

    NASA Astrophysics Data System (ADS)

    Bredeweg, T. A.; Fowler, M. M.; Becker, J. A.; Bond, E. M.; Chadwick, M. B.; Clement, R. R. C.; Esch, E.-I.; Ethvignot, T.; Granier, T.; Jandel, M.; Macri, R. A.; O'Donnell, J. M.; Reifarth, R.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Wouters, J. M.; Wu, C. Y.

    2007-08-01

    We have recently begun a program of high precision measurements of the key production and destruction reactions of important radiochemical diagnostic isotopes, including several isotopes of uranium, plutonium and americium. The detector for advanced neutron capture experiments (DANCE), a 4π BaF2 array located at the Los Alamos Neutron Science Center, will be used to measure the neutron capture cross sections for most of the isotopes of interest. However, neutron capture measurements on many of the actinides are complicated by the presence of prompt γ-rays arising from low energy neutron-induced fission, which competes with neutron capture to varying degrees. Previous measurements of 235U using the DANCE array have shown that we can partially resolve capture from fission events based on total γ-ray calorimetry (i.e. total γ-ray energy versus γ-ray multiplicity). The addition of a dedicated fission-tagging detector to the DANCE array has greatly improved our ability to separate these two competing processes. In addition to higher quality neutron capture data, the addition of a fission-tagging detector offers a means to determine the capture-to-fission ratio (σγ/σf) in a single measurement, which should reduce the effect of systematic uncertainties. We are currently using a dual parallel-plate avalanche counter (PPAC) with the target material electro-deposited directly on the center cathode foil. This design provides a high efficiency for detecting fission fragments and allows loading of pre-assembled target/detector assemblies into the neutron beam line at DANCE. Results from tests of the fission-tag detector, as well as preliminary results from measurements on 235U and 252Cf that utilized the fission-tag detector will be presented.

  2. Fission: The first 50 years

    SciTech Connect

    Vandenbosch, R.

    1989-01-01

    The possibility of fission had been largely unanticipated prior to its discovery in 1938. This process, with its dramatically large energy release and its formation of previously unknown nuclides, immediately captured the imagination of the scientific community. Both theoretical and experimental developments occurred at a rapid pace. I will begin my discussion of fission with the far-reaching paper of Bohr and Wheeler, who in little more than half a year laid out a framework for understanding many features of the fission process. I will then turn to our current understanding of a number of aspects of fission. One of these is the pronounced tendency of many nuclear species to fission asymmetrically. In fact, the discovery of fission was based on the identification of barium isotopes produced in asymmetric fission. The dramatic changes in the preferred mass division and kinetic energy release with the addition of only a few neutrons to the spontaneously fissioning Fermium isotopes will be emphasized. The problem of the dynamics of saddle to scission will be discussed---this is one aspect of fission for which we do not have all the answers. Another dynamical effect to be discussed is the apparent failure of transition state theory at high excitation energies. The role of single particle (shell) effects in enriching the structure if the potential energy surface will be explored. Spontaneously fissioning isomers and intermediate structure resonances will be discussed. The recognition that short-lived fission isomers are superdeformed shape isomers has been followed by the recent observation of superdeformed shape isomers in the rare earth region. 18 refs., 3 figs.

  3. FY04&05 LDRD Final Report Fission Fragment Sputtering

    SciTech Connect

    Ebbinghaus, B; Trelenberg, T; Meier, T; Felter, T; Sturgeon, J; Kuboda, A; Wolfer, B

    2006-02-22

    Fission fragments born within the first 7 {micro}m of the surface of U metal can eject a thousand or more atoms per fission event. Existing data in the literature show that the sputtering yield ranges from 10 to 10,000 atoms per fission event near the surface, but nothing definitive is known about the energy of the sputtered clusters. Experimental packages were constructed allowing the neutron irradiation of natural uranium foils to investigate the amount of material removed per fission event and the kinetic energy distribution of the sputtered atoms. Samples were irradiated but were never analyzed after irradiation. Similar experiments were attempted in a non-radioactive environment using accelerator driven ions in place of fission induced fragments. These experiments showed that tracks produced parallel to the surface (and not perpendicular to the surface) are the primary source of the resulting particulate ejecta. Modeling studies were conducted in parallel with the experimental work. Because the reactor irradiation experiments were not analyzed, data on the energy of the resulting particulate ejecta was not obtained. However, some data was found in the literature on self sputtering of {sup 252}Cf that was used to estimate the velocity and hence the energy of the ejected particulates. Modeling of the data in the literature showed that the energy of the ejecta was much lower than had been anticipated. A mechanism to understand the nature of the ejecta was pursued. Initially it was proposed that the fission fragment imparts its momenta on the electrons which then impart their momenta on the nuclei. Once the nuclei are in motion, the particulate ejecta would result. This initial model was wrong. The error was in the assumption that the secondary electrons impart their momenta directly on the nuclei. Modeling and theoretical considerations showed that the secondary electrons scatter many times before imparting all their momenta. As a result, their energy transfer is

  4. Heavy element fission products on earth

    NASA Astrophysics Data System (ADS)

    Shukoliukov, Iu. A.

    Current data on the products of spontaneous fission in radioactive minerals, lithospheric rocks, and atmosphere are presented. Methods of nuclear geochronology are discussed together with the role of Pu-244 in the isotopic balance of the earth. Natural chain fission reactions are examined with particular reference to the Oklo phenomenon. The discussion covers geological and chemical features of the Oklo deposits, evaluation of the Oklo fission-product data, and prospects for discovering other natural reactors of this type.

  5. Development of prototype induced-fission-based Pu accountancy instrument for safeguards applications.

    PubMed

    Seo, Hee; Lee, Seung Kyu; An, Su Jung; Park, Se-Hwan; Ku, Jeong-Hoe; Menlove, Howard O; Rael, Carlos D; LaFleur, Adrienne M; Browne, Michael C

    2016-09-01

    Prototype safeguards instrument for nuclear material accountancy (NMA) of uranium/transuranic (U/TRU) products that could be produced in a future advanced PWR fuel processing facility has been developed and characterized. This is a new, hybrid neutron measurement system based on fast neutron energy multiplication (FNEM) and passive neutron albedo reactivity (PNAR) methods. The FNEM method is sensitive to the induced fission rate by fast neutrons, while the PNAR method is sensitive to the induced fission rate by thermal neutrons in the sample to be measured. The induced fission rate is proportional to the total amount of fissile material, especially plutonium (Pu), in the U/TRU product; hence, the Pu amount can be calibrated as a function of the induced fission rate, which can be measured using either the FNEM or PNAR method. In the present study, the prototype system was built using six (3)He tubes, and its performance was evaluated for various detector parameters including high-voltage (HV) plateau, efficiency profiles, dead time, and stability. The system's capability to measure the difference in the average neutron energy for the FNEM signature also was evaluated, using AmLi, PuBe, (252)Cf, as well as four Pu-oxide sources each with a different impurity (Al, F, Mg, and B) and producing (α,n) neutrons with different average energies. Future work will measure the hybrid signature (i.e., FNEM×PNAR) for a Pu source with an external interrogating neutron source after enlarging the cavity size of the prototype system to accommodate a large-size Pu source (~600g Pu).

  6. Development of prototype induced-fission-based Pu accountancy instrument for safeguards applications.

    PubMed

    Seo, Hee; Lee, Seung Kyu; An, Su Jung; Park, Se-Hwan; Ku, Jeong-Hoe; Menlove, Howard O; Rael, Carlos D; LaFleur, Adrienne M; Browne, Michael C

    2016-09-01

    Prototype safeguards instrument for nuclear material accountancy (NMA) of uranium/transuranic (U/TRU) products that could be produced in a future advanced PWR fuel processing facility has been developed and characterized. This is a new, hybrid neutron measurement system based on fast neutron energy multiplication (FNEM) and passive neutron albedo reactivity (PNAR) methods. The FNEM method is sensitive to the induced fission rate by fast neutrons, while the PNAR method is sensitive to the induced fission rate by thermal neutrons in the sample to be measured. The induced fission rate is proportional to the total amount of fissile material, especially plutonium (Pu), in the U/TRU product; hence, the Pu amount can be calibrated as a function of the induced fission rate, which can be measured using either the FNEM or PNAR method. In the present study, the prototype system was built using six (3)He tubes, and its performance was evaluated for various detector parameters including high-voltage (HV) plateau, efficiency profiles, dead time, and stability. The system's capability to measure the difference in the average neutron energy for the FNEM signature also was evaluated, using AmLi, PuBe, (252)Cf, as well as four Pu-oxide sources each with a different impurity (Al, F, Mg, and B) and producing (α,n) neutrons with different average energies. Future work will measure the hybrid signature (i.e., FNEM×PNAR) for a Pu source with an external interrogating neutron source after enlarging the cavity size of the prototype system to accommodate a large-size Pu source (~600g Pu). PMID:27337652

  7. The need for precise and well-documented experimental data on prompt fission neutron spectra from neutron-induced fission of 239Pu

    DOE PAGES

    Neudecker, Denise; Taddeucci, Terry Nicholas; Haight, Robert Cameron; Lee, Hye Young; White, Morgan Curtis; Rising, Michael Evans

    2016-01-06

    The spectrum of neutrons emitted promptly after 239Pu(n,f)—a so-called prompt fission neutron spectrum (PFNS)—is a quantity of high interest, for instance, for reactor physics and global security. However, there are only few experimental data sets available that are suitable for evaluations. In addition, some of those data sets differ by more than their 1-σ uncertainty boundaries. We present the results of MCNP studies indicating that these differences are partly caused by underestimated multiple scattering contributions, over-corrected background, and inconsistent deconvolution methods. A detailed uncertainty quantification for suitable experimental data was undertaken including these effects, and test-evaluations were performed with themore » improved uncertainty information. The test-evaluations illustrate that the inadequately estimated effects and detailed uncertainty quantification have an impact on the evaluated PFNS and associated uncertainties as well as the neutron multiplicity of selected critical assemblies. A summary of data and documentation needs to improve the quality of the experimental database is provided based on the results of simulations and test-evaluations. Furthermore, given the possibly substantial distortion of the PFNS by multiple scattering and background effects, special care should be taken to reduce these effects in future measurements, e.g., by measuring the 239Pu PFNS as a ratio to either the 235U or 252Cf PFNS.« less

  8. Fifty years with nuclear fission

    SciTech Connect

    Behrens, J.W.; Carlson, A.D. )

    1989-01-01

    The news of the discovery of nuclear fission, by Otto Hahn and Fritz Strassmann in Germany, was brought to the United States by Niels Bohr in January 1939. Since its discovery, the United States, and the world for that matter, has never been the same. It therefore seemed appropriate to acknowledge the fifieth anniversary of its discovery by holding a topical meeting entitled, Fifty Years with Nuclear Fission,'' in the United States during the year 1989. The objective of the meeting was to bring together pioneers of the nuclear industry and other scientists and engineers to report on reminiscences of the past and on the more recent development in fission science and technology. The conference highlighted the early pioneers of the nuclear industry by dedicated a full day (April 26), consisting of two plenary sessions, at the National Academy of Sciences (NAS) in Washington, DC. More recent developments in fission science and technology in addition to historical reflections were topics for two fully days of sessions (April 27 and 28) at the main site of the NIST in Gaithersburg, Maryland. The wide range of topics covered in this Volume 1 by this topical meeting included plenary invited, and contributed sessions entitled: Preclude to the First Chain Reaction -- 1932 to 1942; Early Fission Research -- Nuclear Structure and Spontaneous Fission; 50 Years of Fission, Science, and Technology; Nuclear Reactors, Secure Energy for the Future; Reactors 1; Fission Science 1; Safeguards and Space Applications; Fission Data; Nuclear Fission -- Its Various Aspects; Theory and Experiments in Support of Theory; Reactors and Safeguards; and General Research, Instrumentation, and By-Product. The individual papers have been cataloged separately.

  9. Theoretical Description of the Fission Process

    SciTech Connect

    Witold Nazarewicz

    2003-07-01

    The main goals of the project can be summarized as follows: Development of effective energy functionals that are appropriate for the description of heavy nuclei. Our goal is to improve the existing energy density (Skyrme) functionals to develop a force that will be used in calculations of fission dynamics. Systematic self-consistent calculations of binding energies and fission barriers of actinide and trans-actinide nuclei using modern density functionals. This will be followed by calculations of spontaneous fission lifetimes and mass and charge divisions using dynamic adiabatic approaches based on the WKB approximation. Investigate novel microscopic (non-adiabatic) methods to study the fission process.

  10. Bimodal Fission in the Skyrme-Hartree-Fock Approach

    SciTech Connect

    Staszczak, A.; Dobaczewski, J.; Nazarewicz, Witold

    2007-01-01

    Spontaneous fission properties of 256Fm, 258Fm, and 260Fm isotopes are studied within the Skyrme-Hartree-Fock+BCS framework. In the particle-hole channel we take the Skyrme SkM* effective force, while in the particle-particle channel we employ the seniority pairing interaction. Three static fission paths for all investigated heavy fermium isotopes are found. The analysis of these fission modes allows to describe observed asymmetric fission of 256Fm, as well as bimodal fission of 258Fm and symmetric fission in 260Fm.

  11. Measurement of {sup 235}U content and flow of UF{sub 6} using delayed neutrons or gamma rays following induced fission

    SciTech Connect

    Stromswold, D.C.; Peurrung, A.J.; Reeder, P.L.; Perkins, R.W.

    1996-06-01

    Feasibility experiments conducted at Pacific Northwest National Laboratory demonstrate that either delayed neutrons or energetic gamma rays from short-lived fission products can be used to monitor the blending of UF{sub 6} gas streams. A {sup 252}Cf neutron source was used to induce {sup 235}U fission in a sample, and delayed neutrons and gamma rays were measured after the sample moved {open_quotes}down-stream.{close_quotes} The experiments used a UO{sub 2} powder that was transported down the pipe to simulate the flowing UF{sub 6} gas. Computer modeling and analytic calculation extended the test results to a flowing UF{sub 6} gas system. Neutron or gamma-ray measurements made at two downstream positions can be used to indicate both the {sup 235}U content and UF{sub 6} flow rate. Both the neutron and gamma-ray techniques have the benefits of simplicity and long-term reliability, combined with adequate sensitivity for low-intrusion monitoring of the blending process. Alternatively, measuring the neutron emission rate from (a, n) reactions in the UF{sub 6} provides an approximate measure of the {sup 235}U content without using a neutron source to induce fission.

  12. Reliability of Monte Carlo simulations in modeling neutron yields from a shielded fission source

    NASA Astrophysics Data System (ADS)

    McArthur, Matthew S.; Rees, Lawrence B.; Czirr, J. Bart

    2016-08-01

    Using the combination of a neutron-sensitive 6Li glass scintillator detector with a neutron-insensitive 7Li glass scintillator detector, we are able to make an accurate measurement of the capture rate of fission neutrons on 6Li. We used this detector with a 252Cf neutron source to measure the effects of both non-borated polyethylene and 5% borated polyethylene shielding on detection rates over a range of shielding thicknesses. Both of these measurements were compared with MCNP calculations to determine how well the calculations reproduced the measurements. When the source is highly shielded, the number of interactions experienced by each neutron prior to arriving at the detector is large, so it is important to compare Monte Carlo modeling with actual experimental measurements. MCNP reproduces the data fairly well, but it does generally underestimate detector efficiency both with and without polyethylene shielding. For non-borated polyethylene it underestimates the measured value by an average of 8%. This increases to an average of 11% for borated polyethylene.

  13. Three-cluster model for the {alpha}-accompanied fission of californium nuclei

    SciTech Connect

    Manimaran, K.; Balasubramaniam, M.

    2009-02-15

    A three-cluster model is proposed to explain the particle-accompanied binary fission of radioactive nuclei. The model is developed as an extension of the preformed cluster model of Gupta and collaborators. The advantage of this model is that, for a fixed third fragment, we can calculate the fragmentation potential minimized in charge coordinate. For our study we chose the various neutron-deficient to neutron-rich californium nuclei, whose analysis reveals that the closed-shell effect of any one of the fragments in ternary fragmentation presents itself as the most favorable configuration to be observed. As one goes from a neutron-deficient to a neutron-rich californium isotope, the role of the neutron closed shell associated with any one of the preferred fragments changes to that of the proton closed shell, and for very neutron rich isotopes of californium the presence of a double closed shell nucleus enhances the decay probability. The quadrupole deformation of the light fragment (A{sub 2}) associated with the preferred configuration in the symmetric mass region also has a transition from positive to negative deformation as one goes from neutron-deficient to neutron-rich californium isotopes. The calculated relative yields of different fragmentation channels are compared with the available experimental yields for {sup 252}Cf.

  14. Dynamical Aspects of Nuclear Fission

    NASA Astrophysics Data System (ADS)

    Kliman, J.; Itkis, M. G.; Gmuca, Š.

    2008-11-01

    Fission dynamics. Dependence of scission-neutron yield on light-fragment mass for [symbol]=1/2 [et al.]. Dynamics of capture quasifission and fusion-fission competition / L. Stuttgé ... [et al.] -- Fission-fission. The processes of fusion-fission and quasi-fission of superheavy nuclei / M. G. Itkis ... [et al.]. Fission and quasifission in the reactions [symbol]Ca+[symbol]Pb and [symbol]Ni+[symbol]W / G. N. Knyazheva ... [et al.]. Mass-energy characteristics of reactions [symbol]Fe+[symbol][symbol][symbol]266Hs and [symbol]Mg+[symbol]Cm[symbol][symbol]Hs at Coulomb barrier / L. Krupa ... [et al.]. Fusion of heavy ions at extreme sub-barrier energies / Ş. Mişicu and H. Esbensen. Fusion and fission dynamics of heavy nuclear system / V. Zagrebaev and W. Greiner. Time-dependent potential energy for fusion and fission processes / A. V. Karpov ... [et al.] -- Superheavy elements. Advances in the understanding of structure and production mechanisms for superheavy elements / W. Greiner and V. Zagrebaev. Fission barriers of heaviest nuclei / A. Sobiczewski ... [et al.]. Possibility of synthesizing doubly magic superheavy nuclei / Y Aritomo ... [et al.]. Synthesis of superheavy nuclei in [symbol]Ca-induced reactions / V. K. Utyonkov ... [et al.] -- Fragmentation. Production of neutron-rich nuclei in the nucleus-nucleus collisions around the Fermi energy / M. Veselský. Signals of enlarged core in [symbol]Al / Y. G. Ma ... [et al.] -- Exotic modes. New insight into the fission process from experiments with relativistic heavy-ion beams / K.-H. Schmidt ... [et al.]. New results for the intensity of bimodal fission in binary and ternary spontaneous fission of [symbol]Cf / C. Goodin ... [et al.]. Rare fission modes: study of multi-cluster decays of actinide nuclei / D. V. Kamanin ... [et al.]. Energy distribution of ternary [symbol]-particles in [symbol]Cf(sf) / M. Mutterer ... [et al.]. Preliminary results of experiment aimed at searching for collinear cluster tripartition of

  15. Nuclear Fission and Fission{minus}Product Spectroscopy: Second International Workshop. Proceedings

    SciTech Connect

    Fioni, G.; Faust, H.; Oberstedt, S.; Hambsch, F.

    1998-10-01

    These proceedings represent papers presented at the Second International Workshop on Nuclear Fission and Fission{minus}Product Spectroscopy held in Seyssins, France in April, 1998. The objective was to bring together the specialists in the field to overview the situation and to assess our present understanding of the fission process. The topics presented at the conference included nuclear waste management, incineration, neutron driven transmutation, leakage etc., radioactive beams, neutron{minus}rich nuclei, neutron{minus}induced and spontaneous fission, ternary fission phenomena, angular momentum, parity and time{minus}reversal phenomena, and nuclear fission at higher excitation energy. Modern spectroscopic tools for gamma spectroscopy as applied to fission were also discussed. There were 53 papers presented at the conference,out of which 3 have been abstracted for the Energy,Science and Technology database.(AIP)

  16. Reflection Asymmetric Shapes in the Neutron-Rich 140,143Ba Isotopes

    NASA Astrophysics Data System (ADS)

    Zhu Sheng-jiang (S, J. Zhu; Wang, Mu-ge; J, H. Hamilton; A, V. Ramayya; B, R. S. Babu; W, C. Ma; Long, Gui-lu; Deng, Jing-kang; Zhu, Ling-yan; Li, Ming; T, N. Ginter; J, Komicki; J, D. Cole; R, Aryaeinejad; Y, K. Dardenne; M, W. Drigert; J, O. Rasmussen; Ts, Yu Oganessian; M, A. Stoyer; S, Y. Chu; K, E. Gregorich; M, F. Mohar; S, G. Prussin; I, Y. Lee; N, R. Johnson; F, K. McGowan

    1997-08-01

    Level schemes for the neutron-rich 140,143Ba nuclei have been determined by study of prompt γ-rays in spontaneous fission of 252Cf. The level pattern and enhanced E1 transitions between π = + and π = - bands show reflection asymmetric shapes with simplex quantum number s = +1 in 140Ba and s = ±i in 143Ba, respectively. The octupole deformation stability with spin variation has been discussed.

  17. Current Issues in Nuclear Data Evaluation Methodology: {sup 235}U Prompt Fission Neutron Spectra and Multiplicity for Thermal Neutrons

    SciTech Connect

    Trkov, A.; Capote, R.; Pronyaev, V.G.

    2015-01-15

    Issues in evaluation methodology of the prompt fission neutron spectra (PFNS) and neutron multiplicity for the thermal-neutron-induced fission of the {sup 235}U are discussed. The inconsistency between the experimental differential and integral data is addressed. By using differential data as ”shape data” good consistency was achieved between available sets of differential data. Integral dosimetry data have been used to define the PFNS slope at high outgoing neutron energies, where the quality of the differential data is poor. The inclusion into the fit of measured integral (spectrum-averaged) cross sections had a very small impact in the region where differential PFNS data are abundant and accurate, but removed the discrepancy with integral data at higher neutron emission energies. All experimental data are consistently fitted giving a PFNS average energy of 2.008 MeV. The impact on criticality prediction of the newly evaluated PFNS was tested. The highly enriched {sup 235}U solution assemblies with high leakage HEU-SOL-THERM-001 and HEU-SOL-THERM-009 benchmarks are the most sensitive to the PFNS. Criticality calculations for those solutions show a significant increase in reactivity if the average neutron energy of the fission neutrons is reduced from the ENDF/B-VI.5 value of 2.03 MeV. The proposed reduction of the PFNS average energy by 1.1% can be compensated by reducing the average number of neutrons per fission ν{sup ¯} at the thermal energy to the Gwin et al. measured value. The simple least-squares PFNS fit was confirmed by a more sophisticated combined fit of differential PFNS data for {sup 233,235}U, {sup 239}Pu and {sup 252}Cf nuclides with the generalised least-squares method using the GMA and GANDR codes.

  18. Fission Spectrum

    DOE R&D Accomplishments Database

    Bloch, F.; Staub, H.

    1943-08-18

    Measurements of the spectrum of the fission neutrons of 25 are described, in which the energy of the neutrons is determined from the ionization produced by individual hydrogen recoils. The slow neutrons producing fission are obtained by slowing down the fast neutrons from the Be-D reaction of the Stanford cyclotron. In order to distinguish between fission neutrons and the remaining fast cyclotron neutrons both the cyclotron current and the pusle amplifier are modulated. A hollow neutron container, in which slow neutrons have a lifetime of about 2 milliseconds, avoids the use of large distances. This method results in much higher intensities than the usual modulation arrangement. The results show a continuous distribution of neutrons with a rather wide maximum at about 0.8 MV falling off to half of its maximum value at 2.0 MV. The total number of netrons is determined by comparison with the number of fission fragments. The result seems to indicate that only about 30% of the neutrons have energies below .8 MV. Various tests are described which were performed in order to rule out modification of the spectrum by inelastic scattering. Decl. May 4, 1951

  19. SPIDER Progress Towards High Resolution Correlated Fission Product Data

    NASA Astrophysics Data System (ADS)

    Shields, Dan; Meierbachtol, Krista; Tovesson, Fredrik; Arnold, Charles; Blackeley, Rick; Bredeweg, Todd; Devlin, Matt; Hecht, Adam; Jandel, Marian; Jorgenson, Justin; Nelson, Ron; White, Morgan; Spider Team

    2014-09-01

    The SPIDER detector (SPectrometer for Ion DEtermination in fission Research) is under development with the goal of obtaining high-resolution, high-efficiency, correlated fission product data needed for many applications including the modeling of next generation nuclear reactors, stockpile stewardship, and the fundamental understanding of the fission process. SPIDER simultaneously measures velocity and energy of both fission products to calculate fission product yields (FPYs), neutron multiplicity (ν), and total kinetic energy (TKE). A detailed description of the prototype SPIDER detector components will be presented. Characterization measurements with alpha and spontaneous fission sources will also be discussed. LA-UR-14-24875. The SPIDER detector (SPectrometer for Ion DEtermination in fission Research) is under development with the goal of obtaining high-resolution, high-efficiency, correlated fission product data needed for many applications including the modeling of next generation nuclear reactors, stockpile stewardship, and the fundamental understanding of the fission process. SPIDER simultaneously measures velocity and energy of both fission products to calculate fission product yields (FPYs), neutron multiplicity (ν), and total kinetic energy (TKE). A detailed description of the prototype SPIDER detector components will be presented. Characterization measurements with alpha and spontaneous fission sources will also be discussed. LA-UR-14-24875. This work is in part supported by LANL Laboratory Directed Research and Development Projects 20110037DR and 20120077DR.

  20. Theoretical Description of the Fission Process

    SciTech Connect

    Witold Nazarewicz

    2009-10-25

    Advanced theoretical methods and high-performance computers may finally unlock the secrets of nuclear fission, a fundamental nuclear decay that is of great relevance to society. In this work, we studied the phenomenon of spontaneous fission using the symmetry-unrestricted nuclear density functional theory (DFT). Our results show that many observed properties of fissioning nuclei can be explained in terms of pathways in multidimensional collective space corresponding to different geometries of fission products. From the calculated collective potential and collective mass, we estimated spontaneous fission half-lives, and good agreement with experimental data was found. We also predicted a new phenomenon of trimodal spontaneous fission for some transfermium isotopes. Our calculations demonstrate that fission barriers of excited superheavy nuclei vary rapidly with particle number, pointing to the importance of shell effects even at large excitation energies. The results are consistent with recent experiments where superheavy elements were created by bombarding an actinide target with 48-calcium; yet even at high excitation energies, sizable fission barriers remained. Not only does this reveal clues about the conditions for creating new elements, it also provides a wider context for understanding other types of fission. Understanding of the fission process is crucial for many areas of science and technology. Fission governs existence of many transuranium elements, including the predicted long-lived superheavy species. In nuclear astrophysics, fission influences the formation of heavy elements on the final stages of the r-process in a very high neutron density environment. Fission applications are numerous. Improved understanding of the fission process will enable scientists to enhance the safety and reliability of the nation’s nuclear stockpile and nuclear reactors. The deployment of a fleet of safe and efficient advanced reactors, which will also minimize radiotoxic

  1. Adiabatic Mass Parameters for Spontaneous Fission

    SciTech Connect

    Baran, A.; Sheikh, J. A.; Nazarewicz, Witold

    2009-01-01

    The collective mass tensor derived from the adiabatic time-dependent Hartree-Fock-Bogoliubov theory, perturbative cranking approximation, and the Gaussian overlap approximation to the generator-coordinate method is discussed. Illustrative calculations are carried out for ^{252}Fm using the nuclear density functional theory with Skyrme interaction SkM* and seniority pairing.

  2. Optimizing moderation of He-3 neutron detectors for shielded fission sources

    DOE PAGES

    Rees, Lawrence B.; Czirr, J. Bart

    2012-07-10

    Abstract: The response of 3-He neutron detectors is highly dependent on the amount of moderator incorporated into the detector system. If there is too little moderation, neutrons will not react with the 3-He. If there is too much moderation, neutrons will not reach the 3-He. In applications for portal or border monitors where 3He detectors are used to interdict illicit Importation of plutonium, the fission source is always shielded to some extent. Since the energy distribution of neutrons emitted from the source depends on the amount and type of shielding present, the optimum placement of moderating material around 3-He tubesmore » is a function of shielding. In this paper, we use Monte Carlo techniques to model the response of 3-He tubes placed in polyethylene boxes for moderation. To model the shielded fission neutron source, we use a 252-Cf source placed in the center of spheres of water of varying radius. Detector efficiency as a function of box geometry and shielding are explored. We find that increasing the amount of moderator behind and to the sides of the detector generally improves the detector response, but that benefits are limited if the thickness of the polyethylene moderator is greater than about 5-7 cm. The thickness of the moderator in front of the 3He tubes, however, is very important. For bare sources, about 5-6 cm of moderator is optimum, but as the shielding increases, the optimum thickness of this moderator decreases to 0-1 cm. A two-tube box with a moderator thickness of 5 cm in front of the first tube and a thickness of 1 cm in front of the second tube is proposed to improve the detector's sensitivity to lower-energy neutrons.« less

  3. Fission meter

    DOEpatents

    Rowland, Mark S.; Snyderman, Neal J.

    2012-04-10

    A neutron detector system for discriminating fissile material from non-fissile material wherein a digital data acquisition unit collects data at high rate, and in real-time processes large volumes of data directly into information that a first responder can use to discriminate materials. The system comprises counting neutrons from the unknown source and detecting excess grouped neutrons to identify fission in the unknown source.

  4. Verification of threshold activation detection (TAD) technique in prompt fission neutron detection using scintillators containing 19F

    NASA Astrophysics Data System (ADS)

    Sibczynski, P.; Kownacki, J.; Moszyński, M.; Iwanowska-Hanke, J.; Syntfeld-Każuch, A.; Gójska, A.; Gierlik, M.; Kaźmierczak, Ł.; Jakubowska, E.; Kędzierski, G.; Kujawiński, Ł.; Wojnarowicz, J.; Carrel, F.; Ledieu, M.; Lainé, F.

    2015-09-01

    In the present study ⌀ 5''× 3'' and ⌀ 2''× 2'' EJ-313 liquid fluorocarbon as well as ⌀ 2'' × 3'' BaF2 scintillators were exposed to neutrons from a 252Cf neutron source and a Sodern Genie 16GT deuterium-tritium (D+T) neutron generator. The scintillators responses to β- particles with maximum endpoint energy of 10.4 MeV from the n+19F reactions were studied. Response of a ⌀ 5'' × 3'' BC-408 plastic scintillator was also studied as a reference. The β- particles are the products of interaction of fast neutrons with 19F which is a component of the EJ-313 and BaF2 scintillators. The method of fast neutron detection via fluorine activation is already known as Threshold Activation Detection (TAD) and was proposed for photofission prompt neutron detection from fissionable and Special Nuclear Materials (SNM) in the field of Homeland Security and Border Monitoring. Measurements of the number of counts between 6.0 and 10.5 MeV with a 252Cf source showed that the relative neutron detection efficiency ratio, defined as epsilonBaF2 / epsilonEJ-313-5'', is 32.0% ± 2.3% and 44.6% ± 3.4% for front-on and side-on orientation of the BaF2, respectively. Moreover, the ⌀ 5'' EJ-313 and side-on oriented BaF2 were also exposed to neutrons from the D+T neutron generator, and the relative efficiency epsilonBaF2 / epsilonEJ-313-5'' was estimated to be 39.3%. Measurements of prompt photofission neutrons with the BaF2 detector by means of data acquisition after irradiation (out-of-beam) of nuclear material and between the beam pulses (beam-off) techniques were also conducted on the 9 MeV LINAC of the SAPHIR facility.

  5. Membrane Fission: Model for Intermediate Structures

    PubMed Central

    Kozlovsky, Yonathan; Kozlov, Michael M.

    2003-01-01

    Membrane budding-fission is a fundamental process generating intracellular carriers of proteins. Earlier works were focused only on formation of coated buds connected to the initial membrane by narrow membrane necks. We present the theoretical analysis of the whole pathway of budding-fission, including the crucial stage where the membrane neck undergoes fission and the carrier separates from the donor membrane. We consider two successive intermediates of the reaction: 1), a constricted membrane neck coming out of aperture of the assembling protein coat, and 2), hemifission intermediate resulting from self-fusion of the inner monolayer of the neck, while its outer monolayer remains continuous. Transformation of the constricted neck into the hemifission intermediate is driven by the membrane stress produced in the neck by the protein coat. Although apparently similar to hemifusion, the fission is predicted to have an opposite dependence on the monolayer spontaneous curvature. Analysis of the further stages of the process demonstrates that in all practically important cases the hemifission intermediate decays spontaneously into two separate membranes, thereby completing the fission process. We formulate the “job description” for fission proteins by calculating the energy they have to deliver and the radii of the protein coat aperture which have to be reached to drive the fission process. PMID:12829467

  6. Monte carlo sampling of fission multiplicity.

    SciTech Connect

    Hendricks, J. S.

    2004-01-01

    Two new methods have been developed for fission multiplicity modeling in Monte Carlo calculations. The traditional method of sampling neutron multiplicity from fission is to sample the number of neutrons above or below the average. For example, if there are 2.7 neutrons per fission, three would be chosen 70% of the time and two would be chosen 30% of the time. For many applications, particularly {sup 3}He coincidence counting, a better estimate of the true number of neutrons per fission is required. Generally, this number is estimated by sampling a Gaussian distribution about the average. However, because the tail of the Gaussian distribution is negative and negative neutrons cannot be produced, a slight positive bias can be found in the average value. For criticality calculations, the result of rejecting the negative neutrons is an increase in k{sub eff} of 0.1% in some cases. For spontaneous fission, where the average number of neutrons emitted from fission is low, the error also can be unacceptably large. If the Gaussian width approaches the average number of fissions, 10% too many fission neutrons are produced by not treating the negative Gaussian tail adequately. The first method to treat the Gaussian tail is to determine a correction offset, which then is subtracted from all sampled values of the number of neutrons produced. This offset depends on the average value for any given fission at any energy and must be computed efficiently at each fission from the non-integrable error function. The second method is to determine a corrected zero point so that all neutrons sampled between zero and the corrected zero point are killed to compensate for the negative Gaussian tail bias. Again, the zero point must be computed efficiently at each fission. Both methods give excellent results with a negligible computing time penalty. It is now possible to include the full effects of fission multiplicity without the negative Gaussian tail bias.

  7. Collinear cluster tripartition channel in the reaction {sup 235}U(n{sub th}, f)

    SciTech Connect

    Pyatkov, Yu. V.; Kamanin, D. V.; Kopach, Yu. N.; Alexandrov, A. A.; Alexandrova, I. A.; Borzakov, S. B.; Voronov, Yu. N.; Zhuchko, V. E.; Kuznetsova, E. A. Panteleev, Ts.; Tyukavkin, A. N.

    2010-08-15

    Investigation of the {sup 235}U(n{sub th}, f) reaction using the miniFOBOS double-arm time-of-flight spectrometer of fission fragments confirmed manifestations of the earlier unknown many-body, at least ternary, decay involving almost collinear decay-product escape, which were first observed in the spontaneous fission of {sup 252}Cf(sf). The use of variables sensitive to the nuclear charge of fission fragments allowed the reliability of identification of decay events to be increased and new decay modes to be revealed.

  8. Spontaneous and induced emission of XeCl* excimer molecules under pumping of Xe – CCl{sub 4} and Ar – Xe – CCl{sub 4} gas mixtures with a low CCl{sub 4} content by fast electrons and uranium fission fragments

    SciTech Connect

    Mis'kevich, A I; Guo, J; Dyuzhov, Yu A

    2013-11-30

    The spontaneous and induced emission of XeCl* excimer molecules upon excitation of Xe – CCl{sub 4} and Ar – Xe – CCl{sub 4} gas mixtures with a low CCl{sub 4} content by high-energy charged particles [a pulsed high-energy electron beam and products of neutron nuclear reaction {sup 235}U(n, f)] has been experimentally studied. The electron energy was 150 keV, and the pump current pulse duration and amplitude were 5 ns and 5 A, respectively. The energy of fission fragments did not exceed 100 MeV, the duration of the neutron pump pulse was 200 μs, and the specific power contribution to the gas was about 300 W cm{sup -3}. Electron beam pumping in a cell 4 cm long with a cavity having an output mirror transmittance of 2.7% gives rise to lasing on the B → X transition in the XeCl* molecule (λ = 308 nm) with a gain α = 0.0085 cm{sup -1} and fluorescence efficiency η ≈ 10%. Pumping by fission fragments in a 250-cm-long cell with a cavity formed by a highly reflecting mirror and a quartz window implements amplified spontaneous emission (ASE) with an output power of 40 – 50 kW sr{sup -1} and a base ASE pulse duration of ∼200 ms. .

  9. Fission Half Lives of Fermium Isotopes Within Skyrme Hartree-Fock Theory

    NASA Astrophysics Data System (ADS)

    Baran, A.; Staszczak, A.; Nazarewicz, W.

    Nuclear fission barriers, mass parameters and spontaneous fission half lives of fermium isotopes calculated in a framework of the Skyrme Hartree-Fock-Bogoliubov model with the SkM* force are discussed. Zero-point energy corrections in the ground state are determined for each nucleus using the Gaussian overlap approximation of the generator coordinate method and in the cranking formalism. Results of spontaneous fission half lives are compared to experimental data.

  10. FISSION HALF LIVES OF FERMIUM ISOTOPES WITHIN SKYRME HARTREE-FOCK-BOGOLIUBOV THEORY

    SciTech Connect

    Baran, A.; Staszczak, Andrzej; Nazarewicz, A.

    2011-01-01

    Nuclear fission barriers, mass parameters and spontaneous fission half lives of fermium isotopes calculated in a framework of the Skyrme Hartree-Fock-Bogoliubov model with the SkM* force are discussed. Zero-point energy corrections in the ground state are determined for each nucleus using the Gaussian overlap approximation of the generator coordinate method and in the cranking formalism. Results of spontaneous fission half lives are compared to experimental data.

  11. Spontaneous Partitioning of Californium from Curium: Curious Cases from the Crystallization of Curium Coordination Complexes

    SciTech Connect

    Cary, Samantha K.; Silver, Mark A.; Liu, Guokui; Wang, Jamie C.; Bogart, Justin A.; Stritzinger, Jared T.; Arico, Alexandra A.; Hanson, Kenneth; Schelter, Eric J.; Albrecht-Schmitt, Thomas E.

    2015-12-07

    The reaction of 248CmCl3 with excess 2,6-pyridinedicarboxylic acid (DPA) under mild solvothermal conditions results in crystallization of the tris-chelate complex Cm(HDPA)3·H2O. Approximately half of the curium remains in solution at the end of this process, and evaporation of the mother liquor results in crystallization of the bis-chelate complex [Cm(HDPA)- (H2DPA)(H2O)2Cl]Cl·2H2O. 248Cm is the daughter of the α decay of 252Cf and is extracted in high purity from this parent. However, trace amounts of 249,250,251Cf are still present in all samples of 248Cm. During the crystallization of Cm(HDPA)3·H2O and [Cm(HDPA)(H2DPA)(H2O)2Cl]Cl·2H2O, californium(III) spontaneously separates itself from the curium complexes and is found doped within crystals of DPA in the form of Cf(HDPA)3. These results add to the growing body of evidence that the chemistry of californium is fundamentally different from that of earlier actinides.

  12. Spontaneous Partitioning of Californium from Curium: Curious Cases from the Crystallization of Curium Coordination Complexes.

    PubMed

    Cary, Samantha K; Silver, Mark A; Liu, Guokui; Wang, Jamie C; Bogart, Justin A; Stritzinger, Jared T; Arico, Alexandra A; Hanson, Kenneth; Schelter, Eric J; Albrecht-Schmitt, Thomas E

    2015-12-01

    The reaction of (248)CmCl3 with excess 2,6-pyridinedicarboxylic acid (DPA) under mild solvothermal conditions results in crystallization of the tris-chelate complex Cm(HDPA)3 · H2O. Approximately half of the curium remains in solution at the end of this process, and evaporation of the mother liquor results in crystallization of the bis-chelate complex [Cm(HDPA)(H2DPA)(H2O)2Cl]Cl·2H2O. (248)Cm is the daughter of the α decay of (252)Cf and is extracted in high purity from this parent. However, trace amounts of (249,250,251)Cf are still present in all samples of (248)Cm. During the crystallization of Cm(HDPA)3 · H2O and [Cm(HDPA)(H2DPA)(H2O)2Cl]Cl · 2H2O, californium(III) spontaneously separates itself from the curium complexes and is found doped within crystals of DPA in the form of Cf(HDPA)3. These results add to the growing body of evidence that the chemistry of californium is fundamentally different from that of earlier actinides.

  13. Synthesis of superheavy element 120 via {sup 50}Ti+{sup A}Cf hot fusion reactions

    SciTech Connect

    Liu, Z. H.; Bao Jingdong

    2009-11-15

    Synthesis of superheavy element 120 in terms of the {sup 50}Ti+{sup 249-252}Cf fusion-evaporation reactions is evaluated and discussed. It is found that the reactions of {sup 250,251}Cf({sup 50}Ti,3n){sup 297,298}120 and {sup 251,252}Cf({sup 50}Ti,4n){sup 297,298}120 are relatively favorable with the maximum evaporation-residue cross sections of 0.12, 0.09, 0.11, and 0.25 pb, respectively. However, {sup 252}Cf may be difficult to be target because its spontaneous fission will bring about serious background in the experiment. Fusion probabilities for different target-projectile combinations leading to the formation of surperheavy nucleus {sup 302}120 are estimated with the ''fusion-by-diffusion'' model and presented as a function of the Coulomb parameter Z{sub 1}Z{sub 2}/(A{sub 1}{sup 1/3}+A{sub 2}{sup 1/3}). Among the reactions {sup 50}Ti+{sup 252}Cf, {sup 54}Cr+{sup 248}Cm, {sup 58}Fe+{sup 244}Pu, and {sup 64}Ni+{sup 238}U, the reaction {sup 50}Ti+{sup 252}Cf has the largest fusion probability. Synthesis of superheavy element 120 is of essential importance for determining whether the magic proton shell should be at Z=114 or at higher proton numbers Z=120-126. Therefore, the experiment to produce isotopes with Z=120 in the fusion reactions {sup 50}Ti+{sup 250,251}Cf is of great interest.

  14. Fifty years with nuclear fission. Volume 1

    SciTech Connect

    Behrens, J.W.; Carlson, A.D.

    1989-12-31

    The news of the discovery of nuclear fission, by Otto Hahn and Fritz Strassmann in Germany, was brought to the United States by Niels Bohr in January 1939. Since its discovery, the United States, and the world for that matter, has never been the same. It therefore seemed appropriate to acknowledge the fifieth anniversary of its discovery by holding a topical meeting entitled, ``Fifty Years with Nuclear Fission,`` in the United States during the year 1989. The objective of the meeting was to bring together pioneers of the nuclear industry and other scientists and engineers to report on reminiscences of the past and on the more recent development in fission science and technology. The conference highlighted the early pioneers of the nuclear industry by dedicated a full day (April 26), consisting of two plenary sessions, at the National Academy of Sciences (NAS) in Washington, DC. More recent developments in fission science and technology in addition to historical reflections were topics for two fully days of sessions (April 27 and 28) at the main site of the NIST in Gaithersburg, Maryland. The wide range of topics covered in this Volume 1 by this topical meeting included plenary invited, and contributed sessions entitled: Preclude to the First Chain Reaction -- 1932 to 1942; Early Fission Research -- Nuclear Structure and Spontaneous Fission; 50 Years of Fission, Science, and Technology; Nuclear Reactors, Secure Energy for the Future; Reactors 1; Fission Science 1; Safeguards and Space Applications; Fission Data; Nuclear Fission -- Its Various Aspects; Theory and Experiments in Support of Theory; Reactors and Safeguards; and General Research, Instrumentation, and By-Product. The individual papers have been cataloged separately.

  15. Capture cross section measurement analysis in the Californium-252 spectrum with the Monte Carlo method.

    PubMed

    Manojlovič, Stanko; Trkov, Andrej; Žerovnik, Gašper; Snoj, Luka

    2015-07-01

    Absolute average capture cross sections of gold, thorium, tantalum, molybdenum, copper and strontium in (252)Cf spontaneous fission neutron spectrum were simulated for two types of experiment setups preformed by Z. Dezso and J. Csikai and by L. Green. The experiments were simulated with MCNP5 using cross section data from the ENDF/B-VII.0 library. The determination of neutron backscattering was calculated with the use of neutron flagging. Correction factors to experimentally measured values were determined to obtain average cross sections in a pure (252)Cf spontaneous fission spectrum. Influence of concrete wall thickness, air moisture and room size on the average cross section was analyzed. Correction factors amounted to about 30%. Corrected values corresponding to average cross sections in a pure (252)Cf spectrum were calculated for (197)Au, (232)Th, (181)Ta, (98)Mo, (65)Cu and (84)Sr. Average cross sections were also calculated with the RR_UNC software using IRDFF-v.1.05 and ENDF/B-VII.0 libraries. The revised average radiative capture cross sections are 75.5±0.1 mb for (197)Au, 87.0±1.6 mb for (232)Th , 98.0±4.5 mb for (181)Ta, 21.2±0.5 mb for (98)Mo, 10.3±0.3 mb for (63)Cu, and 34.9±6.5 mb for (84)Sr.

  16. Seminar on Fission VI

    NASA Astrophysics Data System (ADS)

    Wagemans, Cyriel; Wagemans, Jan; D'Hondt, Pierre

    2008-04-01

    Topical reviews. Angular momentum in fission / F. Gönnenwein ... [et al.]. The processes of fusion-fission and quasi-fission of heavy and super-heavy nuclei / M. G. Itkis ... [et al.] -- Fission cross sections and fragment properties. Minor-actinides fission cross sections and fission fragment mass yields via the surrogate reaction technique / B. Jurado ... [et al.]. Proton-induced fission on actinide nuclei at medium energy / S. Isaev ... [et al.]. Fission cross sections of minor actinides and application in transmutation studies / A. Letourneau ... [et al.]. Systematics on even-odd effects in fission fragments yields: comparison between symmetric and asymmetric splits / F. Rejmund, M Caamano. Measurement of kinetic energy distributions, mass and isotopic yields in the heavy fission products region at Lohengrin / A. Bail ... [et al.] -- Ternary fission. On the Ternary [symbol] spectrum in [symbol]Cf(sf) / M. Mutterer ... [et al.]. Energy degrader technique for light-charged particle spectroscopy at LOHENGRIN / A. Oberstedt, S. Oberstedt, D. Rochman. Ternary fission of Cf isotopes / S. Vermote ... [et al.]. Systematics of the triton and alpha particle emission in ternary fission / C. Wagemans, S. Vermote, O. Serot -- Neutron emission in fission. Scission neutron emission in fission / F.-J. Hambsch ... [et al.]. At and beyond the Scission point: what can we learn from Scission and prompt neutrons? / P. Talou. Fission prompt neutron and gamma multiplicity by statistical decay of fragments / S. Perez-Martin, S. Hilaire, E. Bauge -- Fission theory. Structure and fission properties of actinides with the Gogny force / H. Goutte ... [et al.]. Fission fragment properties from a microscopic approach / N. Dubray, H. Goutte, J.-P. Delaroche. Smoker and non-smoker neutron-induced fission rates / I. Korneev ... [et al.] -- Facilities and detectors. A novel 2v2E spectrometer in Manchester: new development in identification of fission fragments / I. Tsekhanovich ... [et al

  17. Prompt fission gamma-ray studies at DANCE

    SciTech Connect

    Jandel, M.; Rusev, G.; Bond, E. M.; Bredeweg, T. A.; Chadwick, M. B.; Couture, A.; Fowler, M.. M; Haight, R. C.; Kawano, T.; Keksis, A. L.; Mosby, S. M.; O’Donnell, J. M.; Rundberg, R. S.; Stetcu, I.; Talou, P.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Stoyer, M. A.; Haslett, R. J.; Henderson, R. A.; Becker, J. A.; Wu, C. Y.

    2014-11-26

    Measurements of correlated data on prompt-fission γ-rays (PFG) have been carried out for various actinide isotopes in recent years using the Detector for Advanced Neutron Capture Experiments (DANCE) at Los Alamos National Laboratory (LANL). We have developed a model that conveniently parametrizes the correlated data of γ-ray multiplicity and energy. New results on two- dimensional prompt-fission γ-ray multiplicity versus energy distributions from spontaneous fission on ²⁵²Cf and neutron-induced fission on 242mAm are presented together with previously obtained results on 233,235U and ²³⁹Pu. Correlated PFG data from ²⁵²Cf are also compared to results of the detailed theoretical model developed at LANL, for different thresholds of PFG energies. Future plans to measure correlated data on fission fragments, prompt fission neutrons and γ-rays at DANCE are presented.

  18. Fission xenon from extinct Pu-244 in 14,301.

    NASA Technical Reports Server (NTRS)

    Drozd, R.; Hohenberg, C. M.; Ragan, D.

    1972-01-01

    Xenon extracted in step-wise heating of lunar breccia 14,301 contains a fission-like component in excess of that attributable to uranium decay during the age of the solar system. There seems to be no adequate source for this component other than Pu-244. Verification that this component is in fact due to the spontaneous fission of extinct Pu-244 comes from the derived spectrum which is similar to that observed from artificially produced Pu-244. It thus appears that Pu-244 was extant at the time lunar crustal material cooled sufficiently to arrest the thermal diffusion of xenon. Subsequent history has apparently maintained the isotopic integrity of plutonium fission xenon. Of major importance are details of the storage itself. Either the fission component is the result of in situ fission of Pu-244 and subsequent storage in 14,301 material, or the fission xenon was stored in an intermediate reservoir before incorporation into 14,301.

  19. The quantum and thermodynamical characteristics of fission taking into account adiabatic and nonadiabatic modes of motion

    SciTech Connect

    Kadmensky, S. G.

    2007-09-15

    In the framework of the quantum theory of spontaneous and low-energy induced fission, the nature of quantum and thermodynamical properties of a fissioning system is analyzed taking into account adiabatic and nonadiabatic modes of motion for different fission stages. It is shown that, owing to the influence of the Coriolis interaction, the states of the fissile nucleus and of primary fission products are cold and strongly nonequilibrium. The important role of superfluid and pairing nucleon-nucleon correlations for binary and ternary fission is demonstrated. The mechanism of pumping of high values of relative orbital momenta and spins of fission fragments for binary and ternary fission and the nonevaporation mechanism of formation of third particles for ternary fission are investigated. The anisotropies and P-odd, P-even, and T-odd asymmetries for angular distributions of fission products are analyzed.

  20. Use of Neutron Benchmark Fields for the Validation of Dosimetry Cross Sections

    NASA Astrophysics Data System (ADS)

    Griffin, Patrick

    2016-02-01

    The evolution of validation metrics for dosimetry cross sections in neutron benchmark fields is explored. The strength of some of the metrics in providing validation evidence is examined by applying them to the 252Cf spontaneous fission standard neutron benchmark field, the 235U thermal neutron fission reference benchmark field, the ACRR pool-type reactor central cavity reference benchmark fields, and the SPR-III fast burst reactor central cavity. The IRDFF dosimetry cross section library is used in the validation study and observations are made on the amount of coverage provided to the library contents by validation data available in these benchmark fields.

  1. Enhanced trigger for the NIFFTE fissionTPC in presence of high-rate alpha backgrounds

    NASA Astrophysics Data System (ADS)

    Bundgaard, Jeremy; Niffte Collaboration

    2015-10-01

    Nuclear physics and nuclear energy communities call for new, high precision measurements to improve existing fission models and design next generation reactors. The Neutron Induced Fission Fragment Tracking experiment (NIFFTE) has developed the fission Time Projection Chamber (fissionTPC) to measure neutron induced fission with unrivaled precision. The fissionTPC is annually deployed to the Weapons Neutron Research facility at Los Alamos Neutron Science Center where it operates with a neutron beam passing axially through the drift volume, irradiating heavy actinide targets to induce fission. The fissionTPC was developed at the Lawrence Livermore National Laboratory's TPC lab, where it measures spontaneous fission from radioactive sources to characterize detector response, improve performance, and evolve the design. To measure 244Cm, we've developed a fission trigger to reduce the data rate from alpha tracks while maintaining a high fission detection efficiency. In beam, alphas from 239Pu are a large background when detecting fission fragments; implementing the fission trigger will greatly reduce this background. The implementation of the cathode fission trigger in the fissionTPC will be presented along with a detailed study of its efficiency.

  2. Geometry of membrane fission.

    PubMed

    Frolov, Vadim A; Escalada, Artur; Akimov, Sergey A; Shnyrova, Anna V

    2015-01-01

    Cellular membranes define the functional geometry of intracellular space. Formation of new membrane compartments and maintenance of complex organelles require division and disconnection of cellular membranes, a process termed membrane fission. Peripheral membrane proteins generally control membrane remodeling during fission. Local membrane stresses, reflecting molecular geometry of membrane-interacting parts of these proteins, sum up to produce the key membrane geometries of fission: the saddle-shaped neck and hour-glass hemifission intermediate. Here, we review the fundamental principles behind the translation of molecular geometry into membrane shape and topology during fission. We emphasize the central role the membrane insertion of specialized protein domains plays in orchestrating fission in vitro and in cells. We further compare individual to synergistic action of the membrane insertion during fission mediated by individual protein species, proteins complexes or membrane domains. Finally, we describe how local geometry of fission intermediates defines the functional design of the protein complexes catalyzing fission of cellular membranes. PMID:25062896

  3. Fission track length distributions in multi-system thermochronology (Invited)

    NASA Astrophysics Data System (ADS)

    Gleadow, A. J.; Seiler, C.

    2013-12-01

    Fission track length distributions contain a unique record of past temperature variations and therefore play a key role in low-temperature thermochronology, for which there is no exact equivalent in any other method. Confined track lengths closely approximate the true etchable ranges of latent fission tracks [1] and are therefore favoured for fission track studies, but they still have a number of practical limitations. These include small numbers of suitable tracks, especially when only horizontal confined tracks are measured. Using only track-in-track events for measurement further limits the sample size. These restrictions become acute for low track-density samples, where length measurements may be impossible. Irradiating the surface with 252Cf tracks [2] can substantially increase the number of confined tracks, but many researchers do not have access to a Cf source. An even more significant issue has emerged from inter-laboratory comparison experiments that demonstrate a disturbingly poor reproducibility of length measurements between observers [3], a problem compounded by a lack of standardisation in measurement techniques. As a result, individual observers may measure different positions for the end of a track, contributing significantly to variability, and consequently blurring the thermal histories obtained. New digital microscopes open up important opportunities for improved track length measurements by reducing restrictions on sample size, and eliminating some sources of inter-observer bias. We have developed a track length measurement system that enables precise determination of vertical as well as horizontal track dimensions, allowing 3D lengths to be obtained. Lengths are measured on captured image stacks that can be analysed easily and may also be shared, for greater standardisation between laboratories. Length measurements are highly reproducible between different observers using this system, suggesting that at least one source of variability can be

  4. Our 50-year odyssey with fission: Summary

    SciTech Connect

    Nix, J.R.

    1989-01-01

    On the occasion of this International Conference on Fifty Years Research in Nuclear Fission, we summarize our present understanding of the fission process and the challenges that lie ahead. The basic properties of fission arise from a delicate competition between disruptive Coulomb forces, cohesive nuclear forces, and fluctuating shell and pairing forces. These static forces are primarily responsible for such experimental phenomena as deformed ground-state nuclear shapes, fission into fragments of unequal size, sawtooth neutron yields, spontaneously fissioning isomers, broad resonances and narrow intermediate structure in fission cross sections, and cluster radioactivity. However, inertial and dissipative forces also play decisive roles in the dynamical evolution of a fissioning nucleus. The energy dissipated between the saddle and scission points is small for low initial excitation energy at the saddle point and increases with increasing excitation energy. At moderate excitation energies, the dissipation of collective energy into internal single-particle excitation energy proceeds largely through the interaction of nucleons with the mean field and with each other in the vicinity of the nuclear surface, as well as through the transfer of nucleons between the two portions of the evolving dumbell-like system. These unique dissipation mechanisms arise from the Pauli exclusion principle for fermions and the details of the nucleon-nucleon interaction, which make the mean free path of a nucleon near the Fermi surface at low excitation energy longer than the nuclear radius. With its inverse process of heavy-ion fusion reactions, fission continues to yield surprises in the study of large-amplitude collective nuclear motion. 87 refs., 12 figs.

  5. Microscopic Calculations of 240Pu Fission

    SciTech Connect

    Younes, W; Gogny, D

    2007-09-11

    Hartree-Fock-Bogoliubov calculations have been performed with the Gogny finite-range effective interaction for {sup 240}Pu out to scission, using a new code developed at LLNL. A first set of calculations was performed with constrained quadrupole moment along the path of most probable fission, assuming axial symmetry but allowing for the spontaneous breaking of reflection symmetry of the nucleus. At a quadrupole moment of 345 b, the nucleus was found to spontaneously scission into two fragments. A second set of calculations, with all nuclear moments up to hexadecapole constrained, was performed to approach the scission configuration in a controlled manner. Calculated energies, moments, and representative plots of the total nuclear density are shown. The present calculations serve as a proof-of-principle, a blueprint, and starting-point solutions for a planned series of more comprehensive calculations to map out a large set of scission configurations, and the associated fission-fragment properties.

  6. Generalized Energy-Dependent Q Values for Fission

    SciTech Connect

    Vogt, R

    2010-03-31

    We extend Madland's parameterization of the energy release in fission to obtain the dependence of the fission Q value for major and minor actinides on the incident neutron energies in the range 0 {le} E{sub n} {le} 20 MeV. Our parameterization is based on the actinide evaluations recommended for the ENDF/B-VII.1 release. This paper describes the calculation of energydependent fission Q values based on the calculation of the prompt energy release in fission by Madland. This calculation was adopted for use in the LLNL ENDL database and then generalized to obtain the prompt fission energy release for all actinides. Here the calculation is further generalized to the total energy release in fission. There are several stages in a fission event, depending on the time scale. Neutrons and gammas may be emitted at any time during the fission event.While our discussion here is focussed on compound nucleus creation by an incident neutron, similar parameterizations could be obtained for incident gammas or spontaneous fission.

  7. Discovery of a new mode of nuclear fission

    SciTech Connect

    Hulet, E.K.; Wild, J.F.; Dougan, R.J.; Lougheed, R.W.; Landrum, J.H.; Dougan, A.D.; Schaedel, M.; Hahn, R.L.; Baisden, P.A.; Henderson, C.M.

    1986-01-01

    We measured the mass and kinetic-energy partitioning in the spontaneous fission of /sup 258/Fm, /sup 259/Md, /sup 260/Md, /sup 258/No, and /sup 260/(104). Surprisingly, these energy distributions were skewed upward or downward from the peak in each case, except for /sup 260/(104), indicating a composite of two energy distributions. We interpret this as a new mode of fission in which there is mixture of liquid-drop-like and fragment-shell-directed symmetric fission.

  8. Bimodal symmetric fission observed in the heaviest elements

    SciTech Connect

    Hulet, E.K.; Wild, J.F.; Dougan, R.J.; Lougheed, R.W.; Landrum, J.H.; Dougan, A.D.; Schadel, M.; Hahn, R.L.; Baisden, P.A.; Henderson, C.M.

    1986-01-27

    We measured the mass and kinetic-energy partitioning in the spontaneous fission of /sup 258/Fm, /sup 259/Md, /sup 260/Md, /sup 258/No, and /sup 260/(104). All fissioned with mass distributions that were symmetric. Total-kinetic-energy distributions peaked near either 200 or 235 MeV. Surprisingly, these energy distributions were skewed upward or downward from the peak in each case, except for /sup 260/(104), indicating a composite of two energy distributions. We interpret this as a mixture of liquid-drop-like and fragment-shell directed symmetric fission, although theory had not anticipated this phenomenon.

  9. Coupling of the pairing vibrations with the fission mode

    NASA Astrophysics Data System (ADS)

    Staszczak, A.; Baran, A.; Pomorski, K.; Böning, K.

    1985-10-01

    The influence of collective pairing vibrations on the spontaneous fission lifetimes are studied. The Nilsson single-particle potential plus the monopole pairing residual interaction are used. The collective hamiltonian is obtained within the cranking model. The fission lifetimes are evaluated in the WKB approximation along the least-action trajectory in the three-dimensional space (ε 24, Δ p, Δ n) . When taking into account the mean paring-field parameters (Δ p, Δ n) as dynamical variables, the theoretical fission lifetimes decrease by a few orders of magnitude.

  10. Analusis by 252Cf plasma desorption mass spectrometry of Bordetella pertussis endotoxin after nitrous deamination

    NASA Astrophysics Data System (ADS)

    Deprun, C.; Karibian, D.; Caroff, M.

    1993-07-01

    Endotoxic lipopolysaccharides (LPSs) are the major components of Gram-negative bacterial outer membrane. Like many amphipathic molecules, they pose problems of heterogeneity, purity, solubility, and aggregation. Nevertheless, PDMS has recently have been applied to unmodified endotoxins composed of LPS having uip to five sugar units in their saccharide chain. The B. Pertussis LPSs, most of which have a dodecasaccharide domain, ahve been analysed by classical methods and the masses of the separate lipid and saccharide domains determined after rupture of the bond linking them. However, the acid treatment employed for these and most chemical analyses can also modify structures in the vicinity of the bond. In order to investigate this biologically-important region, the endotoxin was treated to nitrous deamination, which shortens the saccharide chain to five sugars, but preserves the acid-labile region of the LPS. The PDM spectrum of this derivative, which required new conditions for its desorption, confirmed the structure analysis and demonstrated the presence of at least four molecular species.

  11. Effect of α-damage on fission-track annealing in zircon

    USGS Publications Warehouse

    Kasuya, Masao; Naeser, Charles W.

    1988-01-01

    The thermal stability of confined fission-track lengths in four zircon samples having different spontaneous track densities (i.e., different amounts of ??-damage) has been studied by one-hour isochronal annealing experiments. The thermal stability of spontaneous track lengths is independent of initial spontaneous track density. The thermal stability of induced track lengths in pre-annealed zircon, however, is significantly higher than that of spontaneous track lengths. The results indicate that the presence of ??-damage lowers the thermal stability of fission-tracks in zircon.

  12. The effect of α-damage on fission-track annealing in zircon

    USGS Publications Warehouse

    Kasuya, M.; Naeser, C.W.

    1988-01-01

    The thermal stability of confined fission-track lengths in four zircon samples having different spontaneous track densities (i.e. different amounts of ??-damage) has been studied by one hour isochronal annealing experiments. The thermal stability of spontaneous track lengths is independent of initial spontaneous track density. The thermal stability of induced track lengths in pre-annealed zircon, however, is significantly higher than that of spontaneous track lengths. The results indicate that the presence of ??-damage lowers the thermal stability of fission-tracks in zircon. ?? 1988.

  13. Fission cross section measurement of Cm-247, Es-254 and Cf-250: Progress report

    SciTech Connect

    Block, R.C.

    1989-03-01

    The Rensselaer Intense Neutron Spectrometer (RINS) system has been activated to measure the fission cross sections of microgram quantities of transuranic nuclei. The fast electronics have been tested with spontaneous fission pulses from the Cf-252-coated electrodes in the fission chamber used for the Cm-242 and Pu-238 measurements by Alam et al.; six chains of electronics, each consisting of a preamplifier, power filter, fast amplifier and fast discriminator, are now working and available to take data. 3 refs.

  14. Resonant tunneling and the bimodal symmetric fission of sup 258 Fm

    SciTech Connect

    Bhandari, B.S. )

    1991-02-25

    The concept of resonant tunneling is invoked to explain the sharp drop in the measured spontaneous-fission half-life when going from {sup 256}Fm to {sup 258}Fm. Various consequences of such a suggestion on the other observed characteristics of the bimodal symmetric fission of {sup 258}Fm are briefly discussed.

  15. Design of a californium-based epithermal neutron beam for neutron capture therapy.

    PubMed

    Yanch, J C; Kim, J K; Wilson, M J

    1993-08-01

    The potential of the spontaneously fissioning isotope, 252Cf, to provide epithermal neutrons for use in boron neutron capture therapy (BNCT) has been investigated using Monte Carlo simulation. The Monte Carlo code MCNP was used to design an assembly composed of a 26 cm long, 11 cm radius cylindrical D2O moderator followed by a 64 cm long Al filter. Lithium filters are placed between the moderator and the filter and between the Al and the patient. A reflector surrounding the moderator/filter assembly is required in order to maintain adequate therapy flux at the patient position. An ellipsoidal phantom composed of skull- and brain-equivalent material was used to determine the dosimetric effect of this beam. It was found that both advantage depths and advantage ratios compare very favourably with reactor and accelerator epithermal neutron sources. The dose rate obtainable, on the other hand, is 4.1 RBE cGy min-1, based on a very large (1.0 g) source of 252Cf. This dose rate is two to five times lower than those provided by existing reactor beams and can be viewed as a drawback of using 252Cf as a neutron source. Radioisotope sources, however, do offer the advantage of in-hospital installation.

  16. The Fission Barrier Landscape

    SciTech Connect

    Phair, L.; Moretto, L. G.

    2008-04-17

    Fission excitation functions have been measured for a chain of neighboring compound nuclei from {sup 207}Po to {sup 212}Po. We present a new analysis which provides a determination of the fission barriers and ground state shell effects with nearly spectroscopic accuracy. The accuracy achieved in this analysis may lead to a future detailed exploration of the saddle mass surface and its spectroscopy.

  17. Fission Spectrum Related Uncertainties

    SciTech Connect

    G. Aliberti; I. Kodeli; G. Palmiotti; M. Salvatores

    2007-10-01

    The paper presents a preliminary uncertainty analysis related to potential uncertainties on the fission spectrum data. Consistent results are shown for a reference fast reactor design configuration and for experimental thermal configurations. However the results obtained indicate the need for further analysis, in particular in terms of fission spectrum uncertainty data assessment.

  18. Fission gas detection system

    DOEpatents

    Colburn, Richard P.

    1985-01-01

    A device for collecting fission gas released by a failed fuel rod which device uses a filter to pass coolant but which filter blocks fission gas bubbles which cannot pass through the filter due to the surface tension of the bubble.

  19. Fission properties and production mechanisms for the heaviest known elements

    SciTech Connect

    Hoffman, D.C.

    1981-01-01

    Mass yields of the spontaneous fission of Fm isotopes, Cf isotopes, and /sup 259/Md are discussed. Actinide yields were measured for bombardments of /sup 248/Cm with /sup 16/O, /sup 18/O, /sup 20/Ne, and /sup 22/Ne. A superheavy product might be produced by bombarding /sup 248/Cm with /sup 48/Ca ions. 12 figures. (DLC)

  20. Mass-asymmetric fission in the 40ca+142Nd reaction

    NASA Astrophysics Data System (ADS)

    Prasad, E.; Hinde, D. J.; Williams, E.; Dasgupta, M.; Carter, I. P.; Cook, K. J.; Jeung, D. Y.; Luong, D. H.; McNeil, S.; Palshetkar, C. S.; Rafferty, D. C.; Simenel, C.; Wakhle, A.; Ramachandran, K.; Khuyagbaatar, J.; Dullmann, Ch. E.; Lommel, B.; Kindler, B.

    2016-09-01

    Shell effects play a major role in fission. Mass-asymmetric fission observed in the spontaneous and low energy fission of actinide nuclei was explained by incorporating the fragment shell properties in liquid drop model. Asymmetric fission has also been observed in the low energy fission of neutron-deficient 180Hg nuclei in recent β-delayed fission experiments. This low-energy β-delayed fission has been explained in terms of strong shell effects in pre-scission configurations associated with the system after capture. Calculations predicted asymmetric fission for heavier Hg isotopes as well, at compound nuclear excitation energy as high as 40 MeV. To explore the evolution of fission fragment mass distribution as a function of neutron and proton numbers and also with excitation energy, fission fragment mass distributions have been measured for the 40Ca+142Nd reaction forming the compound nucleus 182Hg at energies around the capture barrier, using the Heavy Ion Accelerator Facility and CUBE spectrometer at the Australian National University. Mass-asymmetric fission is observed in this reaction at an excitation energy of 33.6 MeV. The results are consistent with the β-delayed fission measurements and indicate the presence of shell effects even at higher exciation energies.

  1. Microscopic theory of nuclear fission: a review

    NASA Astrophysics Data System (ADS)

    Schunck, N.; Robledo, L. M.

    2016-11-01

    This article reviews how nuclear fission is described within nuclear density functional theory. A distinction should be made between spontaneous fission, where half-lives are the main observables and quantum tunnelling the essential concept, and induced fission, where the focus is on fragment properties and explicitly time-dependent approaches are often invoked. Overall, the cornerstone of the density functional theory approach to fission is the energy density functional formalism. The basic tenets of this method, including some well-known tools such as the Hartree–Fock–Bogoliubov (HFB) theory, effective two-body nuclear potentials such as the Skyrme and Gogny force, finite-temperature extensions and beyond mean-field corrections, are presented succinctly. The energy density functional approach is often combined with the hypothesis that the time-scale of the large amplitude collective motion driving the system to fission is slow compared to typical time-scales of nucleons inside the nucleus. In practice, this hypothesis of adiabaticity is implemented by introducing (a few) collective variables and mapping out the many-body Schrödinger equation into a collective Schrödinger-like equation for the nuclear wave-packet. The region of the collective space where the system transitions from one nucleus to two (or more) fragments defines what are called the scission configurations. The inertia tensor that enters the kinetic energy term of the collective Schrödinger-like equation is one of the most essential ingredients of the theory, since it includes the response of the system to small changes in the collective variables. For this reason, the two main approximations used to compute this inertia tensor, the adiabatic time-dependent HFB and the generator coordinate method, are presented in detail, both in their general formulation and in their most common approximations. The collective inertia tensor enters also the Wentzel–Kramers–Brillouin (WKB) formula used to

  2. Collective Band Structures in the Neutron-Rich 107,109Ru Nuclei

    NASA Astrophysics Data System (ADS)

    Zhu, Sheng-jiang; Gan, Cui-yun; J, Hamilton H.; A, Ramayya V.; B, Babu R. S.; M, Sakhaee; W, Ma C.; Long, Gui-lu; Deng, Jing-kang; Zhu, Ling-yan; Li, Ming; Yang, Li-ming; J, Komicki; J, Cole D.; R, Aryaeinejad; Y, Dardenne K.; M, Drigert W.; J, Rasmussen O.; M, Stoyer A.; S, Chu Y.; K, Gregorich E.; M, Mohar F.; S, Prussin G.; I, Lee Y.; N, Johnson R.; F, McGowan K.

    1998-11-01

    The levels in neutron-rich odd-A 107,109Ru nuclei have been investigated by using γ-γ- and γ-γ-γ-coincidence studies of the prompt γ-rays from the spontaneous fission of 252Cf. The ground state bands and the negative parity bands are identified and expanded in both nuclei. Triaxial rotor plus particle model calculations indicate the ground state bands originate from ν(d5/2 + g7/2) quasiparticle configurations and the negative parity bands are from νh11/2 orbital.

  3. Reinvestigation of two-phonon γ-vibrational band in neutron-rich 114Pd

    NASA Astrophysics Data System (ADS)

    Huang, Y.; Zhu, S. J.; Hamilton, J. H.; Ramayya, A. V.; Wang, E. H.; Liu, Y. X.; Sun, Y.; Hwang, J. K.; Xiao, Z. G.; Li, H. J.; Luo, Y. X.; Rasmussen, J. O.; Ter-Akopian, G. M.; Oganessian, Yu. Ts.

    2016-08-01

    The level structure in neutron-rich 114Pd nucleus has been reinvestigated by measuring prompt γ rays emitted in the spontaneous fission of 252Cf. A two-phonon γ-vibrational band built on the 1639.3keV level is observed, which confirms the previous suggestion from a β-decay experiment. Systematical comparison supports the assignment for a two-phonon γ-vibrational band in 114Pd. Triaxial projected shell model calculations for the multi-phonon γ bands of 114Pd are in good agreement with the experimental data.

  4. IDENTIFICATION OF HIGH-SPIN STATES IN NEUTRON-RICH 88,90,92Kr AND 86Se

    SciTech Connect

    J. D. Cole

    2011-08-01

    Level schemes of even-even neutron-rich {sup 88-92}Kr and {sup 86}Se have been investigated by measuring triple-{gamma} coincidence data from the spontaneous fission of {sup 252}Cf with the Gammasphere detector array. The level scheme of {sup 88}Kr has been extended up to 7169 keV state. Several new excited states with new transitions have been identified in {sup 90,92}Kr and {sup 86}Se. Spins and parities have been assigned to levels in these nuclei by following regional systematics and angular correlation measurements. The level structures of the N = 52, 54, Se, Kr, and Sr isotones are discussed.

  5. Evidence for octupole excitations in the odd-odd neutron-rich nucleus {sup 142}Cs

    SciTech Connect

    Liu, S. H.; Hamilton, J. H.; Ramayya, A. V.; Hwang, J. K.; Luo, Y. X.; Rasmussen, J. O.; Zhu, S. J.; Ma, W. C.; Daniel, A. V.; Ter-Akopian, G. M.

    2010-05-15

    High-spin states in the neutron-rich nucleus {sup 142}Cs are reinvestigated from a study of the spontaneous fission of {sup 252}Cf with the Gammasphere detector array. A new level scheme is built and spin-parities are assigned to levels based on angular correlation measurements and systematics. The new structure of {sup 142}Cs is proposed to be related to octupole correlations. The electric dipole moment of {sup 142}Cs is measured and a dramatic decrease of the dipole moments with increasing neutron numbers in the Cs isotopic chain is found.

  6. Nuclear structure of the odd-odd N=85 neutron-rich nucleus {sup 140}Cs

    SciTech Connect

    Liu, S. H.; Hamilton, J. H.; Ramayya, A. V.; Hwang, J. K.; Luo, Y. X.; Rasmussen, J. O.; Daniel, A. V.; Ter-Akopian, G. M.; Zhu, S. J.; Ma, W. C.

    2010-03-15

    High-spin excited states in the neutron-rich nucleus {sup 140}Cs were re-investigated from the spontaneous fission of {sup 252}Cf with the Gammasphere detector array. Seven new transitions at low and moderate spin and 13 at high spin were observed in {sup 140}Cs and the level scheme of {sup 140}Cs was extended to 3794 keV with a new sideband. Spins and parities were assigned to levels based on angular correlation measurements and the systematics in the N=85 isotones.

  7. Spontaneous Recovery

    ERIC Educational Resources Information Center

    Rescorla, Robert A.

    2004-01-01

    Spontaneous recovery from extinction is one of the most basic phenomena of Pavlovian conditioning. Although it can be studied by using a variety of designs, some procedures are better than others for identifying the involvement of underlying learning processes. A wide range of different learning mechanisms has been suggested as being engaged by…

  8. Fission induced plasmas

    NASA Technical Reports Server (NTRS)

    Harries, W. L.

    1977-01-01

    The possibility of creating a plasma from fission fragments was investigated, as well as the probability of utilizing the energy of these particles to create population inversion leading to laser action. Eventually, it is hoped that the same medium could be used for both fissioning and lasing, thus avoiding inefficiences in converting one form of energy to the other. A central problem in understanding a fission induced plasma is to obtain an accurate model of the electron behavior; some calculations are presented to this end. The calculations are simple, providing a compendium of processes for reference.

  9. Nuclear fission of Fm isotopes

    SciTech Connect

    Asano, T.; Wada, T.; Ohta, M.; Chiba, S.

    2010-06-01

    Multi-modal fission has been systematically investigated for the series of isotopes of Fm and Cf. The multi-dimensional Langevin-type stochastic differential equation is used for the dynamical calculation. The primary fission mode changes from mass-asymmetric fission to mass-symmetric fission with the increase of neutron numbers for both Fm and Cf cases.

  10. Compilation of fission product yields Vallecitos Nuclear Center

    SciTech Connect

    Rider, B.F.

    1980-01-01

    This document is the ninth in a series of compilations of fission yield data made at Vallecitos Nuclear Center in which fission yield measurements reported in the open literature and calculated charge distributions have been utilized to produce a recommended set of yields for the known fission products. The original data with reference sources, as well as the recommended yields are presented in tabular form for the fissionable nuclides U-235, Pu-239, Pu-241, and U-233 at thermal neutron energies; for U-235, U-238, Pu-239, and Th-232 at fission spectrum energies; and U-235 and U-238 at 14 MeV. In addition, U-233, U-236, Pu-240, Pu-241, Pu-242, Np-237 at fission spectrum energies; U-233, Pu-239, Th-232 at 14 MeV and Cf-252 spontaneous fission are similarly treated. For 1979 U234F, U237F, Pu249H, U234He, U236He, Pu238F, Am241F, Am243F, Np238F, and Cm242F yields were evaluated. In 1980, Th227T, Th229T, Pa231F, Am241T, Am241H, Am242Mt, Cm245T, Cf249T, Cf251T, and Es254T are also evaluated.

  11. The fissionTPC

    NASA Astrophysics Data System (ADS)

    Heffner, Mike

    2014-03-01

    A new instument to study fission, called the fission TPC, has been constructed to make high accuracy measurements of neutron induced fission cross-sections of the major actinides. Most of the cross sections have been measured over the last 60 years, although improvements in the accuracy of the data appear unlikely with the current technology. A potential breakthrough is the deployment of the Time Projection Chamber (TPC) which was developed within the particle physics community. The NIFFTE collaboration, a group of 7 universities and 4 national laboratories, has undertaken the task of building the first TPC for this purpose. In this talk I will present the fission TPC design, challenges that had to be addressed, and the performance of the detector.

  12. Fission Systems for Mars Exploration

    NASA Technical Reports Server (NTRS)

    Houts, Michael G.; Kim, T.; Dorney, D. J.; Swint, Marion Shayne

    2012-01-01

    Fission systems are used extensively on earth, and 34 such systems have flown in space. The energy density of fission is over 10 million times that of chemical reactions, giving fission the potential to eliminate energy density constraints for many space missions. Potential safety and operational concerns with fission systems are well understood, and strategies exist for affordably developing such systems. By enabling a power-rich environment and highly efficient propulsion, fission systems could enable affordable, sustainable exploration of Mars.

  13. Vector soliton fission.

    PubMed

    Lu, F; Lin, Q; Knox, W H; Agrawal, Govind P

    2004-10-29

    We investigate the vectorial nature of soliton fission in an isotropic nonlinear medium both theoretically and experimentally. As a specific example, we show that supercontinuum generation in a tapered fiber is extremely sensitive to the input state of polarization. Multiple vector solitons generated through soliton fission exhibit different states of elliptical polarization while emitting nonsolitonic radiation with complicated polarization features. Experiments performed with a tapered fiber agree with our theoretical description.

  14. Singlet exciton fission photovoltaics.

    PubMed

    Lee, Jiye; Jadhav, Priya; Reusswig, Philip D; Yost, Shane R; Thompson, Nicholas J; Congreve, Daniel N; Hontz, Eric; Van Voorhis, Troy; Baldo, Marc A

    2013-06-18

    Singlet exciton fission, a process that generates two excitons from a single photon, is perhaps the most efficient of the various multiexciton-generation processes studied to date, offering the potential to increase the efficiency of solar devices. But its unique characteristic, splitting a photogenerated singlet exciton into two dark triplet states, means that the empty absorption region between the singlet and triplet excitons must be filled by adding another material that captures low-energy photons. This has required the development of specialized device architectures. In this Account, we review work to develop devices that harness the theoretical benefits of singlet exciton fission. First, we discuss singlet fission in the archetypal material, pentacene. Pentacene-based photovoltaic devices typically show high external and internal quantum efficiencies. They have enabled researchers to characterize fission, including yield and the impact of competing loss processes, within functional devices. We review in situ probes of singlet fission that modulate the photocurrent using a magnetic field. We also summarize studies of the dissociation of triplet excitons into charge at the pentacene-buckyball (C60) donor-acceptor interface. Multiple independent measurements confirm that pentacene triplet excitons can dissociate at the C60 interface despite their relatively low energy. Because triplet excitons produced by singlet fission each have no more than half the energy of the original photoexcitation, they limit the potential open circuit voltage within a solar cell. Thus, if singlet fission is to increase the overall efficiency of a solar cell and not just double the photocurrent at the cost of halving the voltage, it is necessary to also harvest photons in the absorption gap between the singlet and triplet energies of the singlet fission material. We review two device architectures that attempt this using long-wavelength materials: a three-layer structure that uses

  15. General Description of Fission Observables: GEF Model Code

    NASA Astrophysics Data System (ADS)

    Schmidt, K.-H.; Jurado, B.; Amouroux, C.; Schmitt, C.

    2016-01-01

    The GEF ("GEneral description of Fission observables") model code is documented. It describes the observables for spontaneous fission, neutron-induced fission and, more generally, for fission of a compound nucleus from any other entrance channel, with given excitation energy and angular momentum. The GEF model is applicable for a wide range of isotopes from Z = 80 to Z = 112 and beyond, up to excitation energies of about 100 MeV. The results of the GEF model are compared with fission barriers, fission probabilities, fission-fragment mass- and nuclide distributions, isomeric ratios, total kinetic energies, and prompt-neutron and prompt-gamma yields and energy spectra from neutron-induced and spontaneous fission. Derived properties of delayed neutrons and decay heat are also considered. The GEF model is based on a general approach to nuclear fission that explains a great part of the complex appearance of fission observables on the basis of fundamental laws of physics and general properties of microscopic systems and mathematical objects. The topographic theorem is used to estimate the fission-barrier heights from theoretical macroscopic saddle-point and ground-state masses and experimental ground-state masses. Motivated by the theoretically predicted early localisation of nucleonic wave functions in a necked-in shape, the properties of the relevant fragment shells are extracted. These are used to determine the depths and the widths of the fission valleys corresponding to the different fission channels and to describe the fission-fragment distributions and deformations at scission by a statistical approach. A modified composite nuclear-level-density formula is proposed. It respects some features in the superfluid regime that are in accordance with new experimental findings and with theoretical expectations. These are a constant-temperature behaviour that is consistent with a considerably increased heat capacity and an increased pairing condensation energy that is

  16. Evidence for bimodal fission in the heaviest elements

    SciTech Connect

    Hulet, E.K.; Wild, J.F.; Lougheed, R.W.; Dougan, R.J.; Landrum, J.H.; Dougan, A.D.; Schaedel, M.; Hahn, R.L.; Baisden, P.A.; Henderson, C.M.

    1987-08-01

    We have measured the mass and kinetic-energy partitioning in the spontaneous fission of five heavy nuclides: /sup 258/Fm, /sup 259/Md, /sup 260/Md /sup 258/No, and /sup 260/(104). Each was produced by heavy-ion reactions with either /sup 248/Cm, /sup 249/Bk, or /sup 254/Es targets. Energies of correlated fragments from the isotopes with millisecond half lives, /sup 258/No and /sup 260/(104), were measured on-line by a special rotating-wheel instrument, while the others were determined off-line after mass separation. All fissioned with mass distributions that were symmetric. Total-kinetic-energy distributions peaked near either 200 or 235 MeV. Surprisingly, because only a single Gaussian energy distribution had been observed previously in actinide fission, these energy distributions were skewed upward or downward from the peak in each case, except for /sup 260/(104), indicating a composite of two energy distributions. We were able to fit accurately two Gaussian curves to the gross energy distributions from the four remaining nuclides. From the multiple TKE distributions and the shapes of the mass distributions, we conclude that there is a low-energy fission component with liquid-drop characteristics which is admixed with a much higher-energy component due to closed fragment shells. We now have further evidence for this conclusion from measurements of the neutron multiplicity in the spontaneous fission of /sup 260/Md. 25 refs., 9 figs.

  17. Evidence for bimodal fission in the heaviest elements

    SciTech Connect

    Hulet, E.K.

    1987-12-10

    We have measured the mass and kinetic-energy partitioning in the spontaneous fission of five heavy nuclides: /sup 258/Fm, /sup 259/Md, /sup 260/Md, /sup 258/No, and /sup 260/(104). Each was produced by heavy-ion reactions with either /sup 248/Cm, /sup 249/Bk, or /sup 254/Es targets. Energies of correlated fragments from the isotopes with millisecond half lives, /sup 258/No and /sup 260/(104), were measured on-line by a special rotating-wheel instrument, while the others were determined off-line after mass separation. All fissioned with mass distributions that were symmetric. Total-kinetic-energy distributions peaked near either 200 or 235 MeV. Surprisingly, because only a single Gaussian energy distribution had been observed previously in actinide fission, these energy distributions were skewed upward or downward from the peak in each case, except for /sup 260/(104), indicating a composite of two energy distributions. We were able to fit accurately two Gaussian curves to the gross energy distributions from the four remaining nuclides. From the multiple TKE distributions and the shapes of the mass distributions, we conclude that there is a low-energy fission component with liquid-drop characteristics which is admixed with a much higher-energy component due to closed fragment shells. We now have further evidence for this conclusion from measurements of the neutron multiplicity in the spontaneous fission of /sup 260/Md.

  18. Shape trends and triaxiality in neutron-rich odd-mass Y and Nbisotopes

    SciTech Connect

    Luo, Y.X.; Rasmussen, J.O.; Gelberg, A.; Stefanescu, I.; Hamilton, J.H.; Ramayya, A.V.; Hwang, J.K.; Zhu, S.J.; Gore, P.M.; Fong,D.; Jones, E.F.; Wu, S.C.; Lee, I.Y.; Ginter, T.N.; Ma, W.C.; Ter-Akopian, G.M.; Daniel, A.V.; Stoyer, M.A.; Donangelo, R.

    2004-09-28

    New level schemes of Y and Nb isotopes are proposed based on measurements of prompt gamma rays from 252Cf fission at Gammasphere. Shape trends regarding triaxiality and quadrupole deformations are studied.

  19. Testing actinide fission yield treatment in CINDER90 for use in MCNP6 burnup calculations

    SciTech Connect

    Fensin, Michael Lorne; Umbel, Marissa

    2015-09-18

    Most of the development of the MCNPX/6 burnup capability focused on features that were applied to the Boltzman transport or used to prepare coefficients for use in CINDER90, with little change to CINDER90 or the CINDER90 data. Though a scheme exists for best solving the coupled Boltzman and Bateman equations, the most significant approximation is that the employed nuclear data are correct and complete. Thus, the CINDER90 library file contains 60 different actinide fission yields encompassing 36 fissionable actinides (thermal, fast, high energy and spontaneous fission). Fission reaction data exists for more than 60 actinides and as a result, fission yield data must be approximated for actinides that do not possess fission yield information. Several types of approximations are used for estimating fission yields for actinides which do not possess explicit fission yield data. The objective of this study is to test whether or not certain approximations of fission yield selection have any impact on predictability of major actinides and fission products. Further we assess which other fission products, available in MCNP6 Tier 3, result in the largest difference in production. Because the CINDER90 library file is in ASCII format and therefore easily amendable, we assess reasons for choosing, as well as compare actinide and major fission product prediction for the H. B. Robinson benchmark for, three separate fission yield selection methods: (1) the current CINDER90 library file method (Base); (2) the element method (Element); and (3) the isobar method (Isobar). Results show that the three methods tested result in similar prediction of major actinides, Tc-99 and Cs-137; however, certain fission products resulted in significantly different production depending on the method of choice.

  20. Prompt fission gamma-ray studies at DANCE

    DOE PAGES

    Jandel, M.; Rusev, G.; Bond, E. M.; Bredeweg, T. A.; Chadwick, M. B.; Couture, A.; Fowler, M.. M; Haight, R. C.; Kawano, T.; Keksis, A. L.; et al

    2014-11-26

    Measurements of correlated data on prompt-fission γ-rays (PFG) have been carried out for various actinide isotopes in recent years using the Detector for Advanced Neutron Capture Experiments (DANCE) at Los Alamos National Laboratory (LANL). We have developed a model that conveniently parametrizes the correlated data of γ-ray multiplicity and energy. New results on two- dimensional prompt-fission γ-ray multiplicity versus energy distributions from spontaneous fission on ²⁵²Cf and neutron-induced fission on 242mAm are presented together with previously obtained results on 233,235U and ²³⁹Pu. Correlated PFG data from ²⁵²Cf are also compared to results of the detailed theoretical model developed at LANL,more » for different thresholds of PFG energies. Future plans to measure correlated data on fission fragments, prompt fission neutrons and γ-rays at DANCE are presented.« less

  1. Microscopic Description of Complex Nuclear Decay: Multimodal Fission

    SciTech Connect

    Staszczak, A.; Baran, A.; Dobaczewski, J.; Nazarewicz, Witold

    2009-01-01

    This year marks the 70th anniversary of the discovery of nuclear fission. While there is little question of the societal importance of fission (e.g., to current and future energy needs), our understanding of this process is still fairly rudimentary due to the intricacy of the problem. Theoretically, fission represents an extreme example of the large-amplitude collective motion: the tunneling of a large, self-bound, superfluid system of mutually interacting particles. In this work, we describe a study of spontaneous fission using the self-consistent nuclear density functional theory and state-of-the-art computational tools. We did not impose any symmetry on the mean field so that the nuclear densities were allowed to acquire arbitrary shapes characterized by elongation, reflection-asymmetry, triaxiality, necking, etc. Here we show that the observed half-lives of nuclei undergoing bimodal fission can be explained in terms of competing pathways corresponding to different geometries of fission products. This is an important step in providing a many-body description of fundamental nuclear decay.

  2. Fission modelling with FIFRELIN

    NASA Astrophysics Data System (ADS)

    Litaize, Olivier; Serot, Olivier; Berge, Léonie

    2015-12-01

    The nuclear fission process gives rise to the formation of fission fragments and emission of particles (n,γ , e-) . The particle emission from fragments can be prompt and delayed. We present here the methods used in the FIFRELIN code, which simulates the prompt component of the de-excitation process. The methods are based on phenomenological models associated with macroscopic and/or microscopic ingredients. Input data can be provided by experiment as well as by theory. The fission fragment de-excitation can be performed within Weisskopf (uncoupled neutron and gamma emission) or a Hauser-Feshbach (coupled neutron/gamma emission) statistical theory. We usually consider five free parameters that cannot be provided by theory or experiments in order to describe the initial distributions required by the code. In a first step this set of parameters is chosen to reproduce a very limited set of target observables. In a second step we can increase the statistics to predict all other fission observables such as prompt neutron, gamma and conversion electron spectra but also their distributions as a function of any kind of parameters such as, for instance, the neutron, gamma and electron number distributions, the average prompt neutron multiplicity as a function of fission fragment mass, charge or kinetic energy, and so on. Several results related to different fissioning systems are presented in this work. The goal in the next decade will be i) to replace some macroscopic ingredients or phenomenological models by microscopic calculations when available and reliable, ii) to be a support for experimentalists in the design of detection systems or in the prediction of necessary beam time or count rates with associated statistics when measuring fragments and emitted particle in coincidence iii) extend the model to be able to run a calculation when no experimental input data are available, iv) account for multiple chance fission and gamma emission before fission, v) account for the

  3. Process for treating fission waste

    DOEpatents

    Rohrmann, Charles A.; Wick, Oswald J.

    1983-01-01

    A method is described for the treatment of fission waste. A glass forming agent, a metal oxide, and a reducing agent are mixed with the fission waste and the mixture is heated. After melting, the mixture separates into a glass phase and a metal phase. The glass phase may be used to safely store the fission waste, while the metal phase contains noble metals recovered from the fission waste.

  4. Spontaneous curvature of phosphatidic acid and lysophosphatidic acid.

    PubMed

    Kooijman, Edgar E; Chupin, Vladimir; Fuller, Nola L; Kozlov, Michael M; de Kruijff, Ben; Burger, Koert N J; Rand, Peter R

    2005-02-15

    The formation of phosphatidic acid (PA) from lysophosphatidic acid (LPA), diacylglycerol, or phosphatidylcholine plays a key role in the regulation of intracellular membrane fission events, but the underlying molecular mechanism has not been resolved. A likely possibility is that PA affects local membrane curvature facilitating membrane bending and fission. To examine this possibility, we determined the spontaneous radius of curvature (R(0p)) of PA and LPA, carrying oleoyl fatty acids, using well-established X-ray diffraction methods. We found that, under physiological conditions of pH and salt concentration (pH 7.0, 150 mM NaCl), the R(0p) values of PA and LPA were -46 A and +20 A, respectively. Thus PA has considerable negative spontaneous curvature while LPA has the most positive spontaneous curvature of any membrane lipid measured to date. The further addition of Ca(2+) did not significantly affect lipid spontaneous curvature; however, omitting NaCl from the hydration buffer greatly reduced the spontaneous curvature of PA, turning it into a cylindrically shaped lipid molecule (R(0p) of -1.3 x 10(2) A). Our quantitative data on the spontaneous radius of curvature of PA and LPA at a physiological pH and salt concentration will be instrumental in developing future models of biomembrane fission.

  5. Pulsed Fission Propulsion Concept

    NASA Technical Reports Server (NTRS)

    1999-01-01

    In the 1960's U.S. Government laboratories, under Project Orion, investigated a pulsed nuclear fission propulsion system. Small nuclear pulse units would be sequentially discharged from the aft end of the vehicle. A blast shield and shock absorber system would protect the crew and convert the shock loads into a continuous propusive force.

  6. Pulsed Fission Propulsion Concept

    NASA Technical Reports Server (NTRS)

    1999-01-01

    In the 1960's U.S. Government laboratories, under Project Orion, investigated a pulsed nuclear fission propulsion system. Small nuclear pulse units would be sequentially discharged from the aft end of the vehicle. A blast shield and shock absorber system would protect the crew and convert the shock loads into a continuous propulsive force.

  7. Evaluation and compilation of fission product yields 1993

    SciTech Connect

    England, T.R.; Rider, B.F.

    1995-12-31

    This document is the latest in a series of compilations of fission yield data. Fission yield measurements reported in the open literature and calculated charge distributions have been used to produce a recommended set of yields for the fission products. The original data with reference sources, and the recommended yields axe presented in tabular form. These include many nuclides which fission by neutrons at several energies. These energies include thermal energies (T), fission spectrum energies (F), 14 meV High Energy (H or HE), and spontaneous fission (S), in six sets of ten each. Set A includes U235T, U235F, U235HE, U238F, U238HE, Pu239T, Pu239F, Pu241T, U233T, Th232F. Set B includes U233F, U233HE, U236F, Pu239H, Pu240F, Pu241F, Pu242F, Th232H, Np237F, Cf252S. Set C includes U234F, U237F, Pu240H, U234HE, U236HE, Pu238F, Am241F, Am243F, Np238F, Cm242F. Set D includes Th227T, Th229T, Pa231F, Am241T, Am241H, Am242MT, Cm245T, Cf249T, Cf251T, Es254T. Set E includes Cf250S, Cm244S, Cm248S, Es253S, Fm254S, Fm255T, Fm256S, Np237H, U232T, U238S. Set F includes Cm243T, Cm246S, Cm243F, Cm244F, Cm246F, Cm248F, Pu242H, Np237T, Pu240T, and Pu242T to complete fission product yield evaluations for 60 fissioning systems in all. This report also serves as the primary documentation for the second evaluation of yields in ENDF/B-VI released in 1993.

  8. Neutron Capture and Fission Measurement on ^238Pu at DANCE

    NASA Astrophysics Data System (ADS)

    Chyzh, Andrii; Wu, Ching-Yen; Kwan, Elaine; Henderson, Roger; Gostic, Jolie; Couture, Aaron; Young, Hye; Ullmann, John; O'Donnell, John; Jandel, Marian; Haight, Robert; Bredeweg, Todd

    2012-10-01

    Neutron capture and fission reactions on actinides are important in nuclear engineering and physics. DANCE (Detector for Advanced Neutron Capture Measurement, LANL) combined with PPAC (avalanche technique based fission tagging detector, LLNL) were used to study the neutron capture reactions in ^238Pu. Because of extreme spontaneous α-radioactivity in ^238Pu and associated safety issues, 3 separate experiments were performed in 2010-2012. The 1st measurement was done without fission tagging on a 396-μg thick target. The 2nd one was with PPAC on the same target. The 3rd final measurement was done on a thin target with a mass of 40 μg in order to reduce α-background load on PPAC. This was the first such measurement in a laboratory environment. The absolute ^238Pu(n,γ) cross section is presented together with the prompt γ-ray multiplicity in the ^238Pu(n,f) reaction.

  9. Cold fission description with constant and varying mass asymmetries

    NASA Astrophysics Data System (ADS)

    Duarte, S. B.; Rodríguez, O.; Tavares, O. A. P.; Gonçalves, M.; García, F.; Guzmán, F.

    1998-05-01

    Different descriptions for varying the mass asymmetry in the fragmentation process are used to calculate the cold fission barrier penetrability. The relevance of the appropriate choice for both the description of the prescission phase and inertia coefficient to unify alpha decay, cluster radioactivity, and spontaneous cold fission processes in the same theoretical framework is explicitly shown. We calculate the half-life of all possible partition modes of nuclei of A>200 following the most recent Mass Table by Audi and Wapstra. It is shown that if one uses the description in which the mass asymmetry is maintained constant during the fragmentation process, the experimental half-life values and mass yield of 234U cold fission are satisfactorily reproduced.

  10. A thrust-sheet propulsion concept using fissionable elements

    NASA Technical Reports Server (NTRS)

    Moeckel, W. E.

    1976-01-01

    A space propulsion concept is proposed and analyzed which consists of a thin sheet coated on one side with fissionable material, so that nuclear power is converted directly into propulsive power. Thrust is available both from ejected fission fragments and from thermal radiation. Optimum thicknesses are determined for the active and substrate layers. This concept is shown to have potential mission capability (in terms of velocity increments) superior to that of all other advanced propulsion concepts for which performance estimates are available. A suitable spontaneously fissioning material such as Cf254 could provide an extremely high-performance first stage beyond earth orbit. In contrast with some other advanced nuclear propulsion concepts, there is no minimum size below which this concept is infeasible.

  11. A thrust-sheet propulsion concept using fissionable elements

    NASA Technical Reports Server (NTRS)

    Moeckel, W. E.

    1976-01-01

    A space propulsion concept is proposed and analyzed which consists of a thin sheet coated on one side with fissionable material, so that nuclear power is converted directly into propulsive power. Thrust is available both from ejected fission fragments and from thermal radiation. Optimum thicknesses are determined for the active and substrate layers. This concept is shown to have potential mission capability (in terms of velocity increments) superior to that of all other advanced propulsion concepts for which performance estimates are available. A suitable spontaneously fissioning material such as Cf-254 could provide an extremely high-performance first stage beyond earth orbit. In contrast with some other advanced nuclear propulsion concepts, there is no minimum size below which this concept is infeasible.

  12. Testing actinide fission yield treatment in CINDER90 for use in MCNP6 burnup calculations

    DOE PAGES

    Fensin, Michael Lorne; Umbel, Marissa

    2015-09-18

    Most of the development of the MCNPX/6 burnup capability focused on features that were applied to the Boltzman transport or used to prepare coefficients for use in CINDER90, with little change to CINDER90 or the CINDER90 data. Though a scheme exists for best solving the coupled Boltzman and Bateman equations, the most significant approximation is that the employed nuclear data are correct and complete. Thus, the CINDER90 library file contains 60 different actinide fission yields encompassing 36 fissionable actinides (thermal, fast, high energy and spontaneous fission). Fission reaction data exists for more than 60 actinides and as a result, fissionmore » yield data must be approximated for actinides that do not possess fission yield information. Several types of approximations are used for estimating fission yields for actinides which do not possess explicit fission yield data. The objective of this study is to test whether or not certain approximations of fission yield selection have any impact on predictability of major actinides and fission products. Further we assess which other fission products, available in MCNP6 Tier 3, result in the largest difference in production. Because the CINDER90 library file is in ASCII format and therefore easily amendable, we assess reasons for choosing, as well as compare actinide and major fission product prediction for the H. B. Robinson benchmark for, three separate fission yield selection methods: (1) the current CINDER90 library file method (Base); (2) the element method (Element); and (3) the isobar method (Isobar). Results show that the three methods tested result in similar prediction of major actinides, Tc-99 and Cs-137; however, certain fission products resulted in significantly different production depending on the method of choice.« less

  13. Beta-delayed fission probabilities of transfermium nuclei, involved in the r-process

    NASA Astrophysics Data System (ADS)

    Panov, I.; Lutostansky, Yu; Thielemann, F.-K.

    2016-01-01

    For the nucleosynthesis of heavy and superheavy nuclei fission becomes very important when the r-process runs in a very high neutron density environment. In part, fission is responsible for the formation of heavy nuclei due to the inclusion of fission products as new seed nuclei (fission cycling). More than that, beta-delayed fission, along with spontaneous fission, is responsible in the late stages of the r-process for the suppression of superheavy element yields. For beta-delayed fission probability calculations a model description of the beta-strength- functions is required. Extended theoretical predictions for astro-physical applications were provided long ago, and new predictions also for superheavy nuclei with uptodate nuclear input are needed. For the further extension of data to heavier transactinides the models of strength- functions should be modified, taking into account more complicated level schemes. In our present calculations the strength-function model is based on the quasi-particle approximation of Finite Fermi Systems Theory. The probabilities of beta-delayed fission and beta-delayed neutron emission are calculated for some transfermium neutron-rich nuclei, and the influence of beta-delayed fission upon superheavy element formation is discussed.

  14. Clusterization in Ternary Fission

    NASA Astrophysics Data System (ADS)

    Kamanin, D. V.; Pyatkov, Y. V.

    This lecture notes are devoted to the new kind of ternary decay of low excited heavy nuclei called by us "collinear cluster tri-partition" (CCT) due to the features of the effect observed, namely, decay partners fly away almost collinearly and at least one of them has magic nucleon composition. At the early stage of our work the process of "true ternary fission" (fission of the nucleus into three fragments of comparable masses) was considered to be undiscovered for low excited heavy nuclei. Another possible prototype—three body cluster radioactivity—was also unknown. The most close to the CCT phenomenon, at least cinematically, stands so called "polar emission", but only very light ions (up to isotopes of Be) were observed so far.

  15. SHAPED FISSIONABLE METAL BODIES

    DOEpatents

    Wigner, E.P.; Williamson, R.R.; Young, G.J.

    1958-10-14

    A technique is presented for grooving the surface of fissionable fuel elements so that expansion can take place without damage to the interior structure of the fuel element. The fissionable body tends to develop internal stressing when it is heated internally by the operation of the nuclear reactor and at the same time is subjected to surface cooling by the circulating coolant. By producing a grooved or waffle-like surface texture, the annular lines of tension stress are disrupted at equally spaced intervals by the grooves, thereby relieving the tension stresses in the outer portions of the body while also facilitating the removal of accumulated heat from the interior portion of the fuel element.

  16. [Fission product yields of 60 fissioning reactions]. Final report

    SciTech Connect

    Rider, B.F.

    1995-05-01

    In keeping with the statement of work, I have examined the fission product yields of 60 fissioning reactions. In co-authorship with the UTR (University Technical Representative) Talmadge R. England ``Evaluation and Compilation of Fission Product Yields 1993,`` LA-UR-94-3106(ENDF-349) October, (1994) was published. This is an evaluated set of fission product Yields for use in calculation of decay heat curves with improved accuracy has been prepared. These evaluated yields are based on all known experimental data through 1992. Unmeasured fission product yields are calculated from charge distribution, pairing effects, and isomeric state models developed at Los Alamos National Laboratory. The current evaluation has been distributed as the ENDF/B-VI fission product yield data set.

  17. Fission-induced plasmas

    NASA Technical Reports Server (NTRS)

    Harries, W. L.; Shiu, Y. J.

    1979-01-01

    The possibility of creating a plasma from fission fragments, and to utilize the energy of the particles to create population inversion that would lead to laser action is investigated. An investigation was made of various laser materials which could be used for nuclear-pumped lasing. The most likely candidate for a fissioning material in the gaseous form is uranium hexafluoride - UF6, and experiments were performed to investigate materials that would be compatible with it. One of the central problems in understanding a fission-induced plasma is to obtain a model of the electron behavior, and some preliminary calculations are presented. In particular, the rates of various processes are discussed. A simple intuitive model of the electron energy distribution function is also shown. The results were useful for considering a mathematical model of a nuclear-pumped laser. Next a theoretical model of a (3)He-Ar nuclear-pumped laser is presented. The theory showed good qualitative agreement with the experimental results.

  18. Extended optical model for fission

    DOE PAGES

    Sin, M.; Capote, R.; Herman, M. W.; Trkov, A.

    2016-03-07

    A comprehensive formalism to calculate fission cross sections based on the extension of the optical model for fission is presented. It can be used for description of nuclear reactions on actinides featuring multi-humped fission barriers with partial absorption in the wells and direct transmission through discrete and continuum fission channels. The formalism describes the gross fluctuations observed in the fission probability due to vibrational resonances, and can be easily implemented in existing statistical reaction model codes. The extended optical model for fission is applied for neutron induced fission cross-section calculations on 234,235,238U and 239Pu targets. A triple-humped fission barrier ismore » used for 234,235U(n,f), while a double-humped fission barrier is used for 238U(n,f) and 239Pu(n,f) reactions as predicted by theoretical barrier calculations. The impact of partial damping of class-II/III states, and of direct transmission through discrete and continuum fission channels, is shown to be critical for a proper description of the measured fission cross sections for 234,235,238U(n,f) reactions. The 239Pu(n,f) reaction can be calculated in the complete damping approximation. Calculated cross sections for 235,238U(n,f) and 239Pu(n,f) reactions agree within 3% with the corresponding cross sections derived within the Neutron Standards least-squares fit of available experimental data. Lastly, the extended optical model for fission can be used for both theoretical fission studies and nuclear data evaluation.« less

  19. A compact gas-filled avalanche counter for DANCE

    NASA Astrophysics Data System (ADS)

    Wu, C. Y.; Chyzh, A.; Kwan, E.; Henderson, R. A.; Gostic, J. M.; Carter, D.; Bredeweg, T. A.; Couture, A.; Jandel, M.; Ullmann, J. L.

    2012-12-01

    A compact gas-filled avalanche counter for the detection of fission fragments was developed for a highly segmented 4π γ-ray calorimeter, namely the Detector for Advanced Neutron Capture Experiments located at the Lujan Center of the Los Alamos Neutron Science Center. It has been used successfully for experiments with 235U, 238Pu, 239Pu, and 241Pu isotopes to provide a unique signature to differentiate the fission from the competing neutron-capture reaction channel. It was also used to study the spontaneous fission in 252Cf. The design and performance of this avalanche counter for targets with extreme α-decay rate up to ˜2.4×108/s are described.

  20. A compact gas-filled avalanche counter for DANCE

    DOE PAGES

    Wu, C. Y.; Chyzh, A.; Kwan, E.; Henderson, R. A.; Gostic, J. M.; Carter, D.; Bredeweg, T. A.; Couture, A.; Jandel, M.; Ullmann, J. L.

    2012-08-04

    A compact gas-filled avalanche counter for the detection of fission fragments was developed for a highly segmented 4π γ-ray calorimeter, namely the Detector for Advanced Neutron Capture Experiments located at the Lujan Center of the Los Alamos Neutron Science Center. It has been used successfully for experiments with 235U, 238Pu,239Pu, and 241Pu isotopes to provide a unique signature to differentiate the fission from the competing neutron-capture reaction channel. We also used it to study the spontaneous fission in 252Cf. The design and performance of this avalanche counter for targets with extreme α-decay rate up to ~2.4×108/s are described.

  1. A compact gas-filled avalanche counter for DANCE

    SciTech Connect

    Wu, C. Y.; Chyzh, A.; Kwan, E.; Henderson, R. A.; Gostic, J. M.; Carter, D.; Bredeweg, T. A.; Couture, A.; Jandel, M.; Ullmann, J. L.

    2012-08-04

    A compact gas-filled avalanche counter for the detection of fission fragments was developed for a highly segmented 4π γ-ray calorimeter, namely the Detector for Advanced Neutron Capture Experiments located at the Lujan Center of the Los Alamos Neutron Science Center. It has been used successfully for experiments with 235U, 238Pu,239Pu, and 241Pu isotopes to provide a unique signature to differentiate the fission from the competing neutron-capture reaction channel. We also used it to study the spontaneous fission in 252Cf. The design and performance of this avalanche counter for targets with extreme α-decay rate up to ~2.4×108/s are described.

  2. Modification of apparent fission yields by Chemical Fractionation following Fission (CFF)

    NASA Astrophysics Data System (ADS)

    Hohenberg, Charles; Meshik, Alex

    2008-04-01

    Grain-by-grain studies of the 2 billion year old Oklo natural reactor, using laser micro-extraction^1,2, yield detailed information about Oklo, a water-moderated pulsed reactor, cycle times, total neutron fluence and duration, but it also demonstrates Chemical Fractionation following Fission. In the CFF process, members of an isobaric yield chain with long half-lives are subject to migration before decay can occur. Of particular interest is the 129 isobar where 17 million ^129I can migrate out of the host grain before decay, and iodine compounds are water soluble. This is amply demonstated by the variation of Xe spectra between micron-sized uranium-bearing minerals and adjacent uranium-free minerals. Fission 129 yields for the spontaneous fission of ^238U generally come from measured ^129Xe in pitchblend^2, ores emplaced by aqueous activity, and are incorrect due to the CFF process. ^238U yields for the 131 and 129 chains, reported in Hyde^3, as 0.455 +- .02 and < 0.012, respectively, the latter being anomalously low. ^1A Meshik, C Hohenberg and O Pravdivtesva, PRL 93, 182302 (2004); A Meshik Sci. Am. Nov (2005), 55; ^2E K Hyde, Nucl Prop of Heavy Elements III (1964).

  3. Kinetic energy deficit in the symmetric fission of /sup 259/Md. [Light particle emission in /sup 256/Fm fission

    SciTech Connect

    Hulet, E.K.; Wild, J.F.; Lougheed, R.W.; Baisden, P.A.; Dougan, R.J.; Mustafa, M.G.

    1980-10-01

    The fragment energies of about 725 coincidence events have now been observed in the spontaneous fission (SF) decay of 105-min /sup 259/Md since its discovery in 1977. The fission of /sup 259/Md is characterized by a symmetric mass distribution, similar to those of /sup 258/Fm and /sup 259/Fm, but with a broad total kinetic energy (anti TKE) distribution which peaks at about 195 MeV, in contrast to those of /sup 258/Fm and /sup 259/Fm, for which the anti TKE is about 240 MeV. This kinetic energy deficit, approx. 40 MeV, has been postulated to be due to the emission of hydrogen-like particles by /sup 259/Md at the scission point in a large fraction of the fissions, leaving the residual fissioning nucleus with 100 protons. The residual nucleus would then be able to divide into two ultrastable tin-like fission fragments, but with less kinetic energy than that observed in the SF of /sup 258/Fm and /sup 259/Fm, because of binding-energy losses and a reduction in the Coulomb repulsion of the major fragments. To test this hypothesis, counter-telescope experiments aimed at detecting and identifying these light particles were performed. In 439 SF events 3 + 3 protons of the appropriate energy were observed, too few to account for the kinetic energy deficit in the fission of /sup 259/Md. There seems to be no explanation for this problem within the framework of current fission theory. These results are discussed along with preliminary measurements of light-particle emission in the SF of /sup 256/Fm. 5 figures.

  4. Fission yield measurements at IGISOL

    NASA Astrophysics Data System (ADS)

    Lantz, M.; Al-Adili, A.; Gorelov, D.; Jokinen, A.; Kolhinen, V. S.; Mattera, A.; Moore, I.; Penttilä, H.; Pomp, S.; Prokofiev, A. V.; Rakopoulos, V.; Rinta-Antila, S.; Simutkin, V.; Solders, A.

    2016-06-01

    The fission product yields are an important characteristic of the fission process. In fundamental physics, knowledge of the yield distributions is needed to better understand the fission process. For nuclear energy applications good knowledge of neutroninduced fission-product yields is important for the safe and efficient operation of nuclear power plants. With the Ion Guide Isotope Separator On-Line (IGISOL) technique, products of nuclear reactions are stopped in a buffer gas and then extracted and separated by mass. Thanks to the high resolving power of the JYFLTRAP Penning trap, at University of Jyväskylä, fission products can be isobarically separated, making it possible to measure relative independent fission yields. In some cases it is even possible to resolve isomeric states from the ground state, permitting measurements of isomeric yield ratios. So far the reactions U(p,f) and Th(p,f) have been studied using the IGISOL-JYFLTRAP facility. Recently, a neutron converter target has been developed utilizing the Be(p,xn) reaction. We here present the IGISOL-technique for fission yield measurements and some of the results from the measurements on proton induced fission. We also present the development of the neutron converter target, the characterization of the neutron field and the first tests with neutron-induced fission.

  5. A Fission-Fusion Origin for Life

    NASA Astrophysics Data System (ADS)

    Norris, V.; Raine, D. J.

    1998-10-01

    To develop a comprehensive `cells-first' approach to the origin of life, we propose that protocells form spontaneously and that the fission and fusion of these protocells drives the dynamics of their evolution. The fitness criterion for this evolution is taken to be the the stability (conservation) of domains in the protocellular membrane as determined by non-covalent molecular associations between the amphiphiles of the membrane and a subset of the macromolecules in the protocell. In the presence of a source of free energy the macromolecular content of the protocell (co-)evolves as the result of (domain-dependent) membrane-catalysed polymerisation of the prebiotic constituents delivered to the protocell by fusion. The metabolism of the cell therefore (co-)evolves on a rugged fitness landscape. We indicate how domain evolution with the same fitness criterion can potentially give rise to coding. Membrane domains may therefore provide the link between protocells and the RNA/DNA-world.

  6. Measurement of Fission Product Yields from Fast-Neutron Fission

    NASA Astrophysics Data System (ADS)

    Arnold, C. W.; Bond, E. M.; Bredeweg, T. A.; Fowler, M. M.; Moody, W. A.; Rusev, G.; Vieira, D. J.; Wilhelmy, J. B.; Becker, J. A.; Henderson, R.; Kenneally, J.; Macri, R.; McNabb, D.; Ryan, C.; Sheets, S.; Stoyer, M. A.; Tonchev, A. P.; Bhatia, C.; Bhike, M.; Fallin, B.; Gooden, M. E.; Howell, C. R.; Kelley, J. H.; Tornow, W.

    2014-09-01

    One of the aims of the Stockpile Stewardship Program is a reduction of the uncertainties on fission data used for analyzing nuclear test data [1,2]. Fission products such as 147Nd are convenient for determining fission yields because of their relatively high yield per fission (about 2%) and long half-life (10.98 days). A scientific program for measuring fission product yields from 235U,238U and 239Pu targets as a function of bombarding neutron energy (0.1 to 15 MeV) is currently underway using monoenergetic neutron beams produced at the 10 MV Tandem Accelerator at TUNL. Dual-fission chambers are used to determine the rate of fission in targets during activation. Activated targets are counted in highly shielded HPGe detectors over a period of several weeks to identify decaying fission products. To date, data have been collected at neutron bombarding energies 4.6, 9.0, 14.5 and 14.8 MeV. Experimental methods and data reduction techniques are discussed, and some preliminary results are presented.

  7. Nuclear fission with mean-field instantons

    SciTech Connect

    Skalski, Janusz

    2008-06-15

    We present a description of nuclear spontaneous fission, and generally of quantum tunneling, in terms of instantons, that is, periodic imaginary-time solutions to time-dependent mean-field equations. This description allows comparisons to be made with the more familiar generator coordinate (GCM) and adiabatic time-dependent Hartree-Fock (ATDHF) methods. It is shown that the action functional whose value for the instanton is the quasiclassical estimate of the decay exponent fulfills the minimum principle when additional constraints are imposed on trial fission paths. In analogy with mechanics, these are conditions of energy conservation and the velocity-momentum relations. In the adiabatic limit, the instanton method reduces to the time-odd ATDHF equation, with collective mass including the time-odd Thouless-Valatin term, while the GCM mass completely ignores velocity-momentum relations. This implies that GCM inertia generally overestimates the instanton-related decay rate. The very existence of the minimum principle offers hope for a variational search for instantons. After the inclusion of pairing, the instanton equations and the variational principle can be expressed in terms of the imaginary-time-dependent Hartree-Fock-Bogoliubov (TDHFB) theory. The adiabatic limit of this theory reproduces ATDHFB inertia.

  8. Fission fragment driven neutron source

    DOEpatents

    Miller, Lowell G.; Young, Robert C.; Brugger, Robert M.

    1976-01-01

    Fissionable uranium formed into a foil is bombarded with thermal neutrons in the presence of deuterium-tritium gas. The resulting fission fragments impart energy to accelerate deuterium and tritium particles which in turn provide approximately 14 MeV neutrons by the reactions t(d,n).sup.4 He and d(t,n).sup.4 He.

  9. TREATMENT OF FISSION PRODUCT WASTE

    DOEpatents

    Huff, J.B.

    1959-07-28

    A pyrogenic method of separating nuclear reactor waste solutions containing aluminum and fission products as buring petroleum coke in an underground retort, collecting the easily volatile gases resulting as the first fraction, he uminum chloride as the second fraction, permitting the coke bed to cool and ll contain all the longest lived radioactive fission products in greatly reduced volume.

  10. Ternary fission of nuclei into comparable fragments

    SciTech Connect

    Karpeshin, F. F.

    2015-07-15

    The problem of nuclear fission into three comparable fragments is considered. A mechanism of true ternary fission is proposed. In contrast to sequential fission, where the three fragments arise upon two sequential events of binary fission, the mechanism in question relies on a scenario that originally involves fission into three fragments. This mechanism is driven by a hexadecapole deformation of the fissioning nucleus, in contrast to binary fission associated with quadrupole vibrations of the nuclear surface. The fragment-mass ratios are estimated. The dynamics of formation of collinear fragments and their subsequent motion in opposite directions is traced. The calculated probability of true ternary fission complies with observed values.

  11. Ternary fission of nuclei into comparable fragments

    NASA Astrophysics Data System (ADS)

    Karpeshin, F. F.

    2015-07-01

    The problem of nuclear fission into three comparable fragments is considered. A mechanism of true ternary fission is proposed. In contrast to sequential fission, where the three fragments arise upon two sequential events of binary fission, the mechanism in question relies on a scenario that originally involves fission into three fragments. This mechanism is driven by a hexadecapole deformation of the fissioning nucleus, in contrast to binary fission associated with quadrupole vibrations of the nuclear surface. The fragment-mass ratios are estimated. The dynamics of formation of collinear fragments and their subsequent motion in opposite directions is traced. The calculated probability of true ternary fission complies with observed values.

  12. Nuclear Fission Research at IRMM

    SciTech Connect

    Hambsch, Franz-Josef

    2005-05-24

    The Institute for Reference Materials and Measurements (IRMM) will celebrate its 45th anniversary in 2005. With its 150-MeV Geel Electron Linear Accelerator (GELINA) and 7-MV Van de Graaff accelerator as multi-purpose neutron sources, it served the nuclear physics community for this period.The research in the field of nuclear fission was focused in recent years on both the measurement and calculation of fission cross sections, and the measurement of fission fragment properties.Fission cross sections were determined for 233Pa and 234U; the fission process was studied in the resolved resonance region of 239Pu(n,f) and for 251Cf(nth,f). These measurements derive their interest from accelerator driven systems, the thorium fuel cycle, high temperature reactors, safety issues of current reactors, and basic physics. The measurements are supported by several modeling efforts that aim at improving model codes and nuclear data evaluation.

  13. A threshold for dissipative fission

    SciTech Connect

    Thoennessen, M.; Bertsch, G.F.

    1993-09-21

    The empirical domain of validity of statistical theory is examined as applied to fission data on pre-fission data on pre-fission neutron, charged particle, and {gamma}-ray multiplicities. Systematics are found of the threshold excitation energy for the appearance of nonstatistical fission. From the data on systems with not too high fissility, the relevant phenomenological parameter is the ratio of the threshold temperature T{sub thresh} to the (temperature-dependent) fission barrier height E{sub Bar}(T). The statistical model reproduces the data for T{sub thresh}/E{sub Bar}(T) < 0.26 {plus_minus} 0.05, but underpredicts the multiplicities at higher T{sub thresh}/E{sub Bar}(T) independent of mass and fissility of the systems.

  14. Calculation of Ambient (H*(10)) and Personal (Hp(10)) Dose Equivalent from a 252Cf Neutron Source

    SciTech Connect

    Traub, Richard J.

    2010-03-26

    The purpose of this calculation is to calculate the neutron dose factors for the Sr-Cf-3000 neutron source that is located in the 318 low scatter room (LSR). The dose factors were based on the dose conversion factors published in ICRP-21 Appendix 6, and the Ambient dose equivalent (H*(10)) and Personal dose equivalent (Hp(10)) dose factors published in ICRP Publication 74.

  15. Experimental determination of moisture distributions in fired clay brick using a 252Cf source: a neutron transmission study.

    PubMed

    El Abd, A; Abdel-Monem, A M; Kansouh, W A

    2013-04-01

    A neutron transmission method was proposed to study liquid transport in porous media. It was applied to study water penetration into two kinds of fired clay bricks. The results showed that the diffusion processes in the investigated samples are different. Water diffusivities and capillary absorption coefficients characterizing both the flow process and the brick samples were determined and compared. The proposed method is simple, accurate and reliable in studying water diffusion in porous media, in real time.

  16. Comparison of lipids A of several Salmonella and Escherichia strains by 252Cf plasma desorption mass spectrometry.

    PubMed Central

    Karibian, D; Deprun, C; Caroff, M

    1993-01-01

    Plasma desorption mass spectrometry has recently been used with success to characterize underivatized lipid A preparations: the major molecular species present give signals indicating their masses, from which probable compositions could be inferred by using the overall composition determined by chemical analyses. In the present study, plasma desorption mass spectrometry was used to compare structures in lipid A preparations isolated from several smooth and rough strains of Escherichia and Salmonella species. Preparations isolated from strains of both genera revealed considerable variation in degree of heterogeneity (number of fatty acids and presence or absence of hexadecanoic acid, phosphorylethanolamine, and aminoarabinose). Molecular species usually associated with Salmonella lipid A were found in preparations from Escherichia sp. In addition, preparations from three different batches of lipid A from one strain of Salmonella minnesota showed significant differences in composition. These results demonstrate that preparations used for biological and structural analyses should be defined in terms of their particular molecular constituents and that no generalizations based on analysis of a single preparation should be made. PMID:8491718

  17. On the effect of an error in a standard D2O-moderated 252Cf energy spectrum.

    PubMed

    Cummings, F M

    2009-12-01

    There appears to be an error in the neutron fluence for neutrons with energies between 9 and 10 MeV for the tabulated D2O-moderated Cf source in ISO 8529-1. If the referenced spectrum is used as tabulated, the error contributes a total error to neutron dose values from this source of approximately 3%.

  18. Prompt Fission Neutron Emission in Resonance Fission of 239Pu

    SciTech Connect

    Hambsch, Franz-Josef; Oberstedt, Stephan; Varapai, Natallia; Serot, Olivier

    2005-05-24

    The prompt neutron emission probability from neutron-induced fission in the resonance region is being investigated at the time-of-flight facility GELINA of the IRMM. A double Frisch-gridded ionization chamber is used as a fission-fragment detector. For the data acquisition of both the fission-fragment signals as well as the neutron detector signals the fast digitization technique has been applied. For the neutron detection, large-volume liquid scintillation detectors from the DEMON collaboration are used. A specialized data analysis program taking advantage of the digital filtering technique has been developed to treat the acquired data.Neutron multiplicity investigations for actinides, especially in resonance neutron-induced fission, are rather scarce. They are, however, important for reactor control and safety issues as well as for understanding the basic physics of the fission process. Fission yield measurements on both 235U and 239Pu without prompt neutron emission coincidence have shown that fluctuation of the fission-fragment mass distribution exists from resonance to resonance, larger in the case of 235U. To possibly explain these observations, the question now is whether the prompt neutron multiplicity shows similar fluctuations with resonance energy.

  19. Spontaneous actin dynamics in contractile rings

    NASA Astrophysics Data System (ADS)

    Kruse, Karsten; Wollrab, Viktoria; Thiagarajan, Raghavan; Wald, Anne; Riveline, Daniel

    Networks of polymerizing actin filaments are known to be capable to self-organize into a variety of structures. For example, spontaneous actin polymerization waves have been observed in living cells in a number of circumstances, notably, in crawling neutrophils and slime molds. During later stages of cell division, they can also spontaneously form a contractile ring that will eventually cleave the cell into two daughter cells. We present a framework for describing networks of polymerizing actin filaments, where assembly is regulated by various proteins. It can also include the effects of molecular motors. We show that the molecular processes driven by these proteins can generate various structures that have been observed in contractile rings of fission yeast and mammalian cells. We discuss a possible functional role of each of these patterns. The work was supported by Agence Nationale de la Recherche, France, (ANR-10-LABX-0030-INRT) and by Deutsche Forschungsgemeinschaft through SFB1027.

  20. Organelle fission in eukaryotes.

    PubMed

    Osteryoung, K W

    2001-12-01

    The cellular machineries that power chloroplast and mitochondrial division in eukaryotes carry out the topologically challenging job of constricting and severing these double-membraned organelles. Consistent with their endosymbiotic origins, mitochondria in protists and chloroplasts in photosynthetic eukaryotes have evolved organelle-targeted forms of FtsZ, the prokaryotic ancestor of tubulin, as key components of their fission complexes. In fungi, animals and plants, mitochondria no longer utilize FtsZ for division, but several mitochondrial division proteins that localize to the outer membrane and intermembrane space, including two related to the filament-forming dynamins, have been identified in yeast and animals. Although the reactions that mediate organelle division are not yet understood, recent progress in uncovering the constituents of the organelle division machineries promises rapid advancement in our understanding of the biochemical mechanisms underlying the distinct but related processes of chloroplast and mitochondrial division in eukaryotes.

  1. Fission yeast septation.

    PubMed

    Cortés, Juan C G; Ramos, Mariona; Osumi, Masako; Pérez, Pilar; Ribas, Juan Carlos

    2016-01-01

    In animal cells cytokinesis relies on the contraction of an actomyosin ring that pulls the plasma membrane to create a cleavage furrow, whose ingression finally divides the mother cell into two daughter cells. Fungal cells are surrounded by a tough and flexible structure called cell wall, which is considered to be the functional equivalent of the extracellular matrix in animal cells. Therefore, in addition to cleavage furrow ingression, fungal cytokinesis also requires the centripetal formation of a septum wall structure that develops between the dividing cells, whose genesis must be strictly coordinated with both the actomyosin ring closure and plasma membrane ingression. Here we briefly review what is known about the septum structure and composition in the fission yeast Schizosaccharomyces pombe, the recent progress about the relationship between septum biosynthesis and actomyosin ring constriction, and the importance of the septum and ring in the steady progression of the cleavage furrow. PMID:27574536

  2. Fission yeast septation

    PubMed Central

    Cortés, Juan C. G.; Ramos, Mariona; Osumi, Masako; Pérez, Pilar; Ribas, Juan Carlos

    2016-01-01

    ABSTRACT In animal cells cytokinesis relies on the contraction of an actomyosin ring that pulls the plasma membrane to create a cleavage furrow, whose ingression finally divides the mother cell into two daughter cells. Fungal cells are surrounded by a tough and flexible structure called cell wall, which is considered to be the functional equivalent of the extracellular matrix in animal cells. Therefore, in addition to cleavage furrow ingression, fungal cytokinesis also requires the centripetal formation of a septum wall structure that develops between the dividing cells, whose genesis must be strictly coordinated with both the actomyosin ring closure and plasma membrane ingression. Here we briefly review what is known about the septum structure and composition in the fission yeast Schizosaccharomyces pombe, the recent progress about the relationship between septum biosynthesis and actomyosin ring constriction, and the importance of the septum and ring in the steady progression of the cleavage furrow. PMID:27574536

  3. Fifty years with nuclear fission

    SciTech Connect

    Behrens, J.W.; Carlson, A.D. )

    1989-01-01

    The news of the discovery of nucler fission, by Otto Hahn and Fritz Strassmann in Germany, was brought to the United States by Niels Bohr in January 1939. Since its discovery, the United States, and the world for that matter, has never been the same. It therefore seemed appropriate to acknowledge the fiftieth anniversary of its discovery by holding a topical meeting entitled, Fifty years with nuclear fission,'' in the United States during the year 1989. The objective of the meeting was to bring together pioneers of the nuclear industry and other scientists and engineers to report on reminiscences of the past and on the more recent developments in fission science and technology. The conference highlighted the early pioneers of the nuclear industry by dedicating a full day (April 26), consisting of two plenary sessions, at the National Academy of Sciences (NAS) in Washington, DC. More recent developments in fission science and technology in addition to historical reflections were topics for two full days of sessions (April 27 and 28) at the main sites of the NIST in Gaithersburg, Maryland. The wide range of topics covered by Volume 2 of this topical meeting included plenary invited, and contributed sessions entitled, Nuclear fission -- a prospective; reactors II; fission science II; medical and industrial applications by by-products; reactors and safeguards; general research, instrumentation, and by-products; and fission data, astrophysics, and space applications. The individual papers have been cataloged separately.

  4. Fusion, fission, and quasi-fission using TDHF

    NASA Astrophysics Data System (ADS)

    Umar, Sait; Oberacker, Volker

    2014-03-01

    We study fusion, fission, and quasi-fission reactions using the time-dependent Hartee-Fock (TDHF) approach together with the density-constrained TDHF method for fusion. The only input is the Skyrme NN interaction, there are no adjustable parameters. We discuss the identification of quasi-fission in 40Ca+238U, the scission dynamics in symmetric fission of 264Fm, as well as calculating heavy-ion interaction potentials V (R) , mass parameters M (R) , and total fusion cross sections from light to heavy systems. Some of the effects naturally included in these calculations are: neck formation, mass exchange, internal excitations, deformation effects, as well as nuclear alignment for deformed systems. Supported by DOE grant DE-FG02-96ER40975.

  5. Cluster aspects of binary fission

    NASA Astrophysics Data System (ADS)

    Andreev, A. V.; Adamian, G. G.; Antonenko, N. V.

    2013-04-01

    With the improved scission-point model the mass distributions are calculated for induced fission of different Hg isotopes with even mass numbers A =180, 184, 188, 192, 196, 198. The calculated mass distribution and mean total kinetic energy of fission fragments are in a good agreement with the existing experimental data. The change in the shape of the mass distribution from asymmetric to more symmetric is revealed with increasing A of the fissioning AHg nucleus, and the reactions are proposed to verify this prediction experimentally.

  6. Simulated fissioning of uranium and testing of the fission-track dating method

    USGS Publications Warehouse

    McGee, V.E.; Johnson, N.M.; Naeser, C.W.

    1985-01-01

    A computer program (FTD-SIM) faithfully simulates the fissioning of 238U with time and 235U with neutron dose. The simulation is based on first principles of physics where the fissioning of 238U with the flux of time is described by Ns = ??f 238Ut and the fissioning of 235U with the fluence of neutrons is described by Ni = ??235U??. The Poisson law is used to set the stochastic variation of fissioning within the uranium population. The life history of a given crystal can thus be traced under an infinite variety of age and irradiation conditions. A single dating attempt or up to 500 dating attempts on a given crystal population can be simulated by specifying the age of the crystal population, the size and variation in the areas to be counted, the amount and distribution of uranium, the neutron dose to be used and its variation, and the desired ratio of 238U to 235U. A variety of probability distributions can be applied to uranium and counting-area. The Price and Walker age equation is used to estimate age. The output of FTD-SIM includes the tabulated results of each individual dating attempt (sample) on demand and/or the summary statistics and histograms for multiple dating attempts (samples) including the sampling age. An analysis of the results from FTD-SIM shows that: (1) The external detector method is intrinsically more precise than the population method. (2) For the external detector method a correlation between spontaneous track count, Ns, and induced track count, Ni, results when the population of grains has a stochastic uranium content and/or when the counting areas between grains are stochastic. For the population method no correlation can exist. (3) In the external detector method the sampling distribution of age is independent of the number of grains counted. In the population method the sampling distribution of age is highly dependent on the number of grains counted. (4) Grains with zero-track counts, either in Ns or Ni, are in integral part of

  7. Mechanism of Cytokinetic Contractile Ring Constriction in Fission Yeast

    PubMed Central

    Stachowiak, Matthew R.; Laplante, Caroline; Chin, Harvey F.; Guirao, Boris; Karatekin, Erdem; Pollard, Thomas D.; O’Shaughnessy, Ben

    2014-01-01

    SUMMARY Cytokinesis involves constriction of a contractile actomyosin ring. The mechanisms generating ring tension and setting the constriction rate remain unknown, since the organization of the ring is poorly characterized, its tension was rarely measured, and constriction is coupled to other processes. To isolate ring mechanisms we studied fission yeast protoplasts, where constriction occurs without the cell wall. Exploiting the absence of cell wall and actin cortex, we measured ring tension and imaged ring organization, which was dynamic and disordered. Computer simulations based on the amounts and biochemical properties of the key proteins showed that they spontaneously self-organize into a tension-generating bundle. Together with rapid component turnover, the self-organization mechanism continuously reassembles and remodels the constricting ring. Ring constriction depended on cell shape, revealing that the ring operates close to conditions of isometric tension. Thus, the fission yeast ring sets its own tension, but other processes set the constriction rate. PMID:24914559

  8. Neutron Emission in Fission and Quasi-Fission

    NASA Astrophysics Data System (ADS)

    Itkis, I.; Bogatchev, A. A.; Chizhov, A. Yu.; Itkis, M. G.; Kliman, J.; Knyazheva, G. N.; Kondratiev, N. A.; Kozulin, E. M.; Korzyukov, I. V.; Krupa, L.; Oganessian, Yu. Ts.; Pokrovski, I. V.; Prokhorova, E. V.; Sagaidak, R. N.; Voskressenski, V. M.; Rusanov, A. Ya.; Corradi, L.; Stefanini, A. M.; Trotta, M.; Beghini, S.; Montagnoli, G.; Scarlassara, F.; Chubarian, G.; Hanappe, F.; Materna, T.; Dorvaux, O.; Rowley, N.; Stuttge, L.; Giardina, G.

    2005-09-01

    The work presents the results of the study of characteristics of the neutron emission in fission and quasi-fission of heavy and super-heavy nuclei, produced in the reactions with heavy ions. These experiments have been performed at the U-400 accelerator of the Flerov Laboratory of Nuclear Reactions (JINR), tandem accelerator in Legnaro (LNL) and VIVITRON accelerator in Strasbourg (IReS) with the use of the time-of-flight spectrometer of fission fragments CORSET and neutron multidetector DEMON. Mass-energy distributions (MED) of the 48Ca + 168Er, 208Pb, 238U and 18O + 208Pb reactions products at energies close to and below the Coulomb barrier have been studied. The pre- and post-fission neutron multiplicities as a function of the fragment mass have been obtained. A significant yield of the asymmetric component observed in the fragment mass distributions in the case of 18O + 208Pb reaction denotes the multimodal nature of the fission process. At the same time an increase in the yield of fragment masses ML ≅ 75-85 and MH ≅ 200-210 in the case 48Ca+208Pb, 238U reactions and ML ≅ 75-85 and MH ≅ 130-140 in the case 48Ca+168Er is rather connected with a quasi-fission process. The obtained neutron multiplicities dependences on fragment masses showed the validity of these assumptions.

  9. Microscopic description of fission in neutron-rich radium isotopes with the Gogny energy density functional

    NASA Astrophysics Data System (ADS)

    Rodrıguez-Guzmán, R.; Robledo, L. M.

    2016-01-01

    Mean-field calculations, based on the D1S, D1N and D1M parametrizations of the Gogny energy density functional, have been carried out to obtain the potential energy surfaces relevant to fission in several Ra isotopes with the neutron number 144≤ N≤ 176. Inner and outer barrier heights as well as first and second isomer excitation energies are given. The existence of a well-developed third minimum along the fission paths of Ra nuclei is analyzed in terms of the energetics of the "fragments" defining such elongated configuration. The masses and charges of the fission fragments are studied as functions of the neutron number in the parent Ra isotope. The comparison between fission and α -decay half-lives, reveals that the former becomes faster for increasing neutron numbers. Though there exists a strong variance of the results with respect to the parameters used in the computation of the spontaneous fission rate, a change in tendency is observed at N=164 with a steady increase that makes heavier neutron-rich Ra isotopes stable against fission, diminishing the importance of fission recycling in the r-process.

  10. Rapid disappearance of shell effects in the fission of transfermium nuclei

    SciTech Connect

    Hulet, E.K.

    1983-01-01

    In the last fifteen years we have learned that nuclear shells have a very broad and pervasive impact on the fission process. In the first few decades after the discovery of nuclear fission, the nucleus was treated as a drop of liquid with smoothly varying attractive and repulsive forces. Although this model still forms the underlying basis for fission, we also observe large effects from the superimposition of shell corrections derived from coupling the quantum states of individual nucleons. The consequences of single-particle coupling on the fission process can be striking and may often overshadow that originating from the intrinsic liquid-drop component. Here, we point out several major features attributable to shell effects in the spontaneous fission (SF) of the lighter actinides, the sudden transition to symmetric fission in the fermium isotopes, and finally new experimental information indicating another transition in the SF of transfermium nuclides due to the disappearance of shell perturbations. In each transition, the abruptness is surprising, and for the moment, such rapid changes in fission behavior lack a theoretical rationale.

  11. Analysis of the scintillation mechanism in a pressurized {sup 4}He fast neutron detector using pulse shape fitting

    SciTech Connect

    Kelley, R.P. Ray, H.; Jordan, K.A.; Murer, D.

    2015-03-15

    An empirical investigation of the scintillation mechanism in a pressurized {sup 4}He gas fast neutron detector was conducted using pulse shape fitting. Scintillation signals from neutron interactions were measured and averaged to produce a single generic neutron pulse shape from both a {sup 252}Cf spontaneous fission source and a (d,d) neutron generator. An expression for light output over time was then developed by treating the decay of helium excited states in the same manner as the decay of radioactive isotopes. This pulse shape expression was fitted to the measured neutron pulse shape using a least-squares optimization algorithm, allowing an empirical analysis of the mechanism of scintillation inside the {sup 4}He detector. A further understanding of this mechanism in the {sup 4}He detector will advance the use of this system as a neutron spectrometer. For {sup 252}Cf neutrons, the triplet and singlet time constants were found to be 970 ns and 686 ns, respectively. For neutrons from the (d,d) generator, the time constants were found to be 884 ns and 636 ns. Differences were noted in the magnitude of these parameters compared to previously published data, however the general relationships were noted to be the same and checked with expected trends from theory. Of the excited helium states produced from a {sup 252}Cf neutron interaction, 76% were found to be born as triplet states, similar to the result from the neutron generator of 71%. The two sources yielded similar pulse shapes despite having very different neutron energy spectra, validating the robustness of the fits across various neutron energies.

  12. Fission of rotating fermium isotopes

    NASA Astrophysics Data System (ADS)

    Baran, A.; Staszczak, A.

    2014-05-01

    In this paper we discuss the process of fission of even fermium isotopes, on the basis of their rotational states. The nuclear intrinsic vorticity and its coupling to the global rotation of the nucleus are used to simulate the interaction between the rotational motion and the pairing field, and lead to pairing quenching in the case of higher angular momentum states. The rotation leads to a decreasing of the fission barrier heights. The ingredients of the model—ground state fission barriers, pairing correlation energies and the cranking moments of inertia—are obtained within the self-consistent Hartree-Fock-Bogoliubov framework using the Skyrme \\text{Sk}{{\\text{M}}^{*}} energy density functional. Fission barriers and half-lives are estimated for spins I up to I = 16ℏ.

  13. Mass measurements near the r-process path using the Canadian Penning Trap mass spectrometer

    NASA Astrophysics Data System (ADS)

    Van Schelt, J.; Lascar, D.; Savard, G.; Clark, J. A.; Caldwell, S.; Chaudhuri, A.; Fallis, J.; Greene, J. P.; Levand, A. F.; Li, G.; Sharma, K. S.; Sternberg, M. G.; Sun, T.; Zabransky, B. J.

    2012-04-01

    The masses of 40 neutron-rich nuclides from Z=51 to 64 were measured at an average precision of δm/m=10-7 using the Canadian Penning Trap mass spectrometer at Argonne National Laboratory. The measurements, of fission fragments from a 252Cf spontaneous fission source in a helium gas catcher, approach the predicted path of the astrophysical r process. Where overlap exists, this data set is largely consistent with previous measurements from Penning traps, storage rings, and reaction energetics, but large systematic deviations are apparent in β-endpoint measurements. Differences in mass excess from the 2003 Atomic Mass Evaluation of up to 400 keV are seen, as well as systematic disagreement with various mass models.

  14. The binary fission origin of the moon

    NASA Technical Reports Server (NTRS)

    Binder, Alan B.

    1986-01-01

    The major arguments for and against the binary fission model of lunar origin are reviewed. Unresolved problems include: (1) how the protoearth acquired sufficient angular velocity to fission, and (2) how the earth-moon system lost its excess angular momentum after fission. Despite these uncertainties, the compositional similarities between the earth's mantle and the bulk moon suggest that the fission model is worth considering. The proposed sequence of events in the formation of the moon by binary fission is given.

  15. Advanced Space Fission Propulsion Systems

    NASA Technical Reports Server (NTRS)

    Houts, Michael G.; Borowski, Stanley K.

    2010-01-01

    Fission has been considered for in-space propulsion since the 1940s. Nuclear Thermal Propulsion (NTP) systems underwent extensive development from 1955-1973, completing 20 full power ground tests and achieving specific impulses nearly twice that of the best chemical propulsion systems. Space fission power systems (which may eventually enable Nuclear Electric Propulsion) have been flown in space by both the United States and the Former Soviet Union. Fission is the most developed and understood of the nuclear propulsion options (e.g. fission, fusion, antimatter, etc.), and fission has enjoyed tremendous terrestrial success for nearly 7 decades. Current space nuclear research and technology efforts are focused on devising and developing first generation systems that are safe, reliable and affordable. For propulsion, the focus is on nuclear thermal rockets that build on technologies and systems developed and tested under the Rover/NERVA and related programs from the Apollo era. NTP Affordability is achieved through use of previously developed fuels and materials, modern analytical techniques and test strategies, and development of a small engine for ground and flight technology demonstration. Initial NTP systems will be capable of achieving an Isp of 900 s at a relatively high thrust-to-weight ratio. The development and use of first generation space fission power and propulsion systems will provide new, game changing capabilities for NASA. In addition, development and use of these systems will provide the foundation for developing extremely advanced power and propulsion systems capable of routinely and affordably accessing any point in the solar system. The energy density of fissile fuel (8 x 10(exp 13) Joules/kg) is more than adequate for enabling extensive exploration and utilization of the solar system. For space fission propulsion systems, the key is converting the virtually unlimited energy of fission into thrust at the desired specific impulse and thrust

  16. The Microscopic Theory of Fission

    SciTech Connect

    Younes, W; Gogny, D

    2009-06-09

    Fission-fragment properties have been calculated for thermal neutron-induced fission on a {sup 239}Pu target, using constrained Hartree-Fock-Bogoliubov calculations with a finite-range effective interaction. A quantitative criterion based on the interaction energy between the nascent fragments is introduced to define the scission configurations. The validity of this criterion is benchmarked against experimental measurements of the kinetic energies and of multiplicities of neutrons emitted by the fragments.

  17. Fission Modes of Mercury Isotopes

    SciTech Connect

    Warda, M.; Staszczak, A.; Nazarewicz, Witold

    2012-01-01

    Background: Recent experiments on -delayed fission in the mercury-lead region and the discovery of asymmetric fission in 180Hg [A. N. Andreyev et al., Phys. Rev. Lett. 105, 252502 (2010)] have stimulated theoretical interest in the mechanism of fission in heavy nuclei.

    Purpose: We study fission modes and fusion valleys in 180Hg and 198Hg to reveal the role of shell effects in the prescission region and explain the experimentally observed fragment mass asymmetry and its variation with A.

    Methods: We use the self-consistent nuclear density functional theory employing Skyrme and Gogny energy density functionals.

    Results: The potential energy surfaces in multidimensional space of collective coordinates, including elongation, triaxiality, reflection-asymmetry, and necking, are calculated for 180Hg and 198Hg. The asymmetric fission valleys well separated from fusion valleys associated with nearly spherical fragments are found in both cases. The density distributions at scission configurations are studied and related to the experimentally observed mass splits.

    Conclusions: The energy density functionals SkM and D1S give a very consistent description of the fission process in 180Hg and 198Hg. We predict a transition from asymmetric fission in 180Hg toward a more symmetric distribution of fission fragments in 198Hg. For 180Hg, both models yield 100Ru/80Kr as the most probable split. For 198Hg, the most likely split is 108Ru/90Kr in HFB-D1S and 110Ru/88Kr in HFB-SkM .

  18. Fusion and fission of fluid amphiphilic bilayers.

    PubMed

    Gotter, Martin; Strey, Reinhard; Olsson, Ulf; Wennerström, Håkan

    2005-01-01

    The system water-oil (n-decane)-nonionic surfactant (C12E5) forms bilayer phases in a large concentration region, but, for a given oil-to-surfactant ratio, only in a narrow temperature range. In addition to the anisotropic lamellar phase (Lalpha) there is also, at slightly higher temperature, a sponge or L3-phase where the bilayers build up an isotropic structure extending macroscopically in three dimensions. In this phase the bilayer mid-surface has a mean curvature close to zero and a negative Euler characteristic. In this paper we study how the bilayers in the lamellar and the sponge phase respond dynamically to sudden temperature changes. The monolayer spontaneous curvature depends sensitively on temperature and a change of temperature thus provides a driving force for a change in bilayer topology. The equilibration therefore involves kinetic steps of fusion/fission of bilayers. Such dynamic processes have previously been monitored by temperature jump experiments using light scattering in the sponge phase. These experiments revealed an extraordinarily strong dependence of the relaxation time on the bilayer volume fraction phi. At phi < 0.1 the relaxation times are so slow that experiments using deuterium nuclear magnetic resonance (2H-NMR) appear feasible. We here report on the first experiments concerned with the dynamics of the macroscopic phase transition sponge-lamellae by 2H-NMR. We find that the sponge-to-lamellae transition occurs through a nucleation process followed by domain growth involving bilayer fission at domain boundaries. In contrast, the lamellae-to-sponge transformation apparently occurs through a succession of uncorrelated bilayer fusion events. PMID:15715316

  19. Neutron Emission in Fission And Quasi-Fission of Hs

    SciTech Connect

    Itkis, I. M.; Itkis, M. G.; Knyazheva, G. N.; Kozulin, E. M.; Krupa, L.; Hanappe, F.; Dorvaux, O.; Stuttge, L.

    2010-04-30

    Mass and energy distributions of fission-like fragments obtained in the reactions {sup 26}Mg+{sup 248}Cm, {sup 36}S+{sup 238}U and {sup 58}Fe+{sup 208}Pb leading to the formation of {sup 266,274}Hs are reported. From the analysis of TKE distributions for symmetric fragment it was found that at energies below the Coulomb barrier the bimodal fission of {sup 274}Hs, formed in the reaction {sup 26}Mg+{sup 248}Cm, is observed, while in the reaction {sup 36}S+{sup 238}U at these energies the main part of the symmetric fragments arises from the quasi-fission process. At energies above the Coulomb barrier the fusion-fission is a main process leading to the formation of symmetric fragment for the both reactions. In the case of {sup 58}Fe+{sup 208}Pb reaction the quasi-fission process is the main reaction mechanism at all measured energies. The pre- and post-scission neutron multiplicities as a function of the fragment mass have been obtained for all studied reactions.

  20. A physics investigation of deadtime losses in neutron counting at low rates with Cf252

    SciTech Connect

    Evans, Louise G; Croft, Stephen

    2009-01-01

    {sup 252}Cf spontaneous fission sources are used for the characterization of neutron counters and the determination of calibration parameters; including both neutron coincidence counting (NCC) and neutron multiplicity deadtime (DT) parameters. Even at low event rates, temporally-correlated neutron counting using {sup 252}Cf suffers a deadtime effect. Meaning that in contrast to counting a random neutron source (e.g. AmLi to a close approximation), DT losses do not vanish in the low rate limit. This is because neutrons are emitted from spontaneous fission events in time-correlated 'bursts', and are detected over a short period commensurate with their lifetime in the detector (characterized by the system die-away time, {tau}). Thus, even when detected neutron events from different spontaneous fissions are unlikely to overlap in time, neutron events within the detected 'burst' are subject to intrinsic DT losses. Intrinsic DT losses for dilute Pu will be lower since the multiplicity distribution is softer, but real items also experience self-multiplication which can increase the 'size' of the bursts. Traditional NCC DT correction methods do not include the intrinsic (within burst) losses. We have proposed new forms of the traditional NCC Singles and Doubles DT correction factors. In this work, we apply Monte Carlo neutron pulse train analysis to investigate the functional form of the deadtime correction factors for an updating deadtime. Modeling is based on a high efficiency {sup 3}He neutron counter with short die-away time, representing an ideal {sup 3}He based detection system. The physics of dead time losses at low rates is explored and presented. It is observed that new forms are applicable and offer more accurate correction than the traditional forms.

  1. Ternary Fission of {sup 249}Cf(n,f) and {sup 250}Cf(SF)

    SciTech Connect

    University of Gent, B-9000 Gent, Belgium; CEA Cadarache, F-13108 Saint-Paul-lez-Durance, France; Institute Laue-Langevin, F-38042 Grenoble, France; EC-JRC Institute for Reference Materials and Measurements, B-2440 Geel, Belgium; Wadsworth Center, New York State Department of Health, Albany NY 12201, USA; Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA; Vermote, S.; Wagemans, C.; Serot, O.; Soldner, T.; Geltenbort, P.; Gils, J. Van; Almahamid, I.; Tian, G.; Rao, L.

    2011-09-01

    During the last years, several Cm and Cf isotopes have been studied by our research group in the frame of a systematic investigation of gas emission characteristics in ternary fission. Here we report on new results on the energy distribution and the emission probability of {sup 3}H, {sup 4}He and {sup 6}He particles emitted in the spontaneous ternary fission of {sup 250}Cf (E{sub exc} = 0 MeV) and in the neutron induced ternary fission of {sup 249}Cf (E{sub exc} = 6.625 MeV). Both measurements were performed using suited and well-calibrated ΔE-E telescope detectors, at the IRMM (Geel, Belgium) for the spontaneous fission and at the very intense neutron beam PF1b at the Institute Laue-Langevin (Grenoble, France) for the neutron induced fission measurement. In this way, the existing database can be enlarged with new results for Z=98 isotopes, which is important for the systematic investigation. Moreover, the investigation of the 'isotope couple' {sup 249}Cf(n,f) - {sup 250}Cf(SF), together with corresponding data for other isotopes, will yield valuable information on the influence of the excitation energy on the particle emission probabilities.

  2. Unusually low fragment energies in the symmetric fission of /sup 259/Md

    SciTech Connect

    Wild, J.F.; Hulet, E.K.; Lougheed, R.W.; Baisden, P.A.; Landrum, J.H.; Dougan, R.J.; Mustafa, M.G.

    1982-10-01

    The 103-min isotope /sup 259/Md has been identified as the daughter of an electron-capture decay branch of /sup 259/No produced via the /sup 248/Cm(/sup 18/O,..cap alpha..3n) reaction. Chemical separations were used to confirm the identity of /sup 259/Md, which decays by spontaneous fission. The kinetic energies of coincident fission fragments were measured, corresponding to a fragment mass which is highly symmetric, similar to those of /sup 258/Fm and /sup 259/Fm. However, the total kinetic energy distribution for /sup 259/Md is considerably broader (FWHM approx.60 MeV) than those of /sup 258/Fm and /sup 259/Fm, and peaks at 201 MeV, about 35--40 MeV lower in energy. Furthermore, the maximum total Kinetic energy of 215 MeV for mass-symmetric events is about 30 MeV lower than for similar events from the spontaneous fission of /sup 258/Fm and /sup 259/Fm. A hypothesis that this energy difference resulted from the emission of light, hydrogen-like particles at scission in a large fraction of /sup 259/Md spontaneous fission decays was shown to be unfounded. From experiments to observe such particles with counter telescopes, an upper limit of 5% was determined for the fraction of fission events accompanied by light-particle emission. The total kinetic energy deficit at mass symmetry must, therefore, be distributed between internal excitation energy and fragment deformation energy at scission. Although the presence of a large amount of fragment deformation energy seems incompatible with symmetric fission into spherical Sn-like fragments, we prefer this explanation because the low total kinetic energy suggests a lowered Coulomb energy resulting from greater separation of the charge centers of deformed fragments at scission.

  3. Compact fission counter for DANCE

    SciTech Connect

    Wu, C Y; Chyzh, A; Kwan, E; Henderson, R; Gostic, J; Carter, D; Bredeweg, T; Couture, A; Jandel, M; Ullmann, J

    2010-11-06

    The Detector for Advanced Neutron Capture Experiments (DANCE) consists of 160 BF{sub 2} crystals with equal solid-angle coverage. DANCE is a 4{pi} {gamma}-ray calorimeter and designed to study the neutron-capture reactions on small quantities of radioactive and rare stable nuclei. These reactions are important for the radiochemistry applications and modeling the element production in stars. The recognition of capture event is made by the summed {gamma}-ray energy which is equivalent of the reaction Q-value and unique for a given capture reaction. For a selective group of actinides, where the neutron-induced fission reaction competes favorably with the neutron capture reaction, additional signature is needed to distinguish between fission and capture {gamma} rays for the DANCE measurement. This can be accomplished by introducing a detector system to tag fission fragments and thus establish a unique signature for the fission event. Once this system is implemented, one has the opportunity to study not only the capture but also fission reactions. A parallel-plate avalanche counter (PPAC) has many advantages for the detection of heavy charged particles such as fission fragments. These include fast timing, resistance to radiation damage, and tolerance of high counting rate. A PPAC also can be tuned to be insensitive to {alpha} particles, which is important for experiments with {alpha}-emitting actinides. Therefore, a PPAC is an ideal detector for experiments requiring a fast and clean trigger for fission. A PPAC with an ingenious design was fabricated in 2006 by integrating amplifiers into the target assembly. However, this counter was proved to be unsuitable for this application because of issues related to the stability of amplifiers and the ability to separate fission fragments from {alpha}'s. Therefore, a new design is needed. A LLNL proposal to develop a new PPAC for DANCE was funded by NA22 in FY09. The design goal is to minimize the mass for the proposed counter

  4. Thorium-uranium fission radiography

    NASA Technical Reports Server (NTRS)

    Haines, E. L.; Weiss, J. R.; Burnett, D. S.; Woolum, D. S.

    1976-01-01

    Results are described for studies designed to develop routine methods for in-situ measurement of the abundance of Th and U on a microscale in heterogeneous samples, especially rocks, using the secondary high-energy neutron flux developed when the 650 MeV proton beam of an accelerator is stopped in a 42 x 42 cm diam Cu cylinder. Irradiations were performed at three different locations in a rabbit tube in the beam stop area, and thick metal foils of Bi, Th, and natural U as well as polished silicate glasses of known U and Th contents were used as targets and were placed in contact with mica which served as a fission track detector. In many cases both bare and Cd-covered detectors were exposed. The exposed mica samples were etched in 48% HF and the fission tracks counted by conventional transmitted light microscopy. Relative fission cross sections are examined, along with absolute Th track production rates, interaction tracks, and a comparison of measured and calculated fission rates. The practicality of fast neutron radiography revealed by experiments to data is discussed primarily for Th/U measurements, and mixtures of other fissionable nuclei are briefly considered.

  5. Fission prompt gamma-ray multiplicity distribution measurements and simulations at DANCE

    SciTech Connect

    Chyzh, A; Wu, C Y; Ullmann, J; Jandel, M; Bredeweg, T; Couture, A; Norman, E

    2010-08-24

    The nearly energy independence of the DANCE efficiency and multiplicity response to {gamma} rays makes it possible to measure the prompt {gamma}-ray multiplicity distribution in fission. We demonstrate this unique capability of DANCE through the comparison of {gamma}-ray energy and multiplicity distribution between the measurement and numerical simulation for three radioactive sources {sup 22}Na, {sup 60}Co, and {sup 88}Y. The prospect for measuring the {gamma}-ray multiplicity distribution for both spontaneous and neutron-induced fission is discussed.

  6. DOSE PROFILE MODELING OF IDAHO NATIONAL LABORATORY’S ACTIVE NEUTRON INTERROGATION TEST FACILITY

    SciTech Connect

    D. L. Chichester; E. H. Seabury; J. M. Zabriskie; J. Wharton; A. J. Caffrey

    2009-06-01

    A new research and development laboratory has been commissioned at Idaho National Laboratory for performing active neutron interrogation research and development. The facility is designed to provide radiation shielding for DT fusion (14.1 MeV) neutron generators (2 x 108 neutrons per second), DD fusion (2.5 MeV) neutron generators (up to 2 x 106 neutrons per second), and 252Cf spontaneous fission neutron sources (6.7 x 107 neutrons per second, 30 micrograms). Shielding at the laboratory is comprised of modular concrete shield blocks 0.76 m thick with tongue-in-groove features to prevent radiation streaming, arranged into one small and one large test vault. The larger vault is designed to allow operation of the DT generator and has walls 3.8 m tall, an entrance maze, and a fully integrated electrical interlock system; the smaller test vault is designed for 252Cf and DD neutron sources and has walls 1.9 m tall and a simple entrance maze. Both analytical calculations and numerical simulations were used in the design process for the building to assess the performance of the shielding walls and to ensure external dose rates are within required facility limits. Dose rate contour plots have been generated for the facility to visualize the effectiveness of the shield wall and entrance maze and to illustrate the spatial profile of the radiation dose field above the facility and the effects of skyshine around the vaults.

  7. Fast-neutron spectrometry using a ³He ionization chamber and digital pulse shape analysis.

    PubMed

    Chichester, D L; Johnson, J T; Seabury, E H

    2012-08-01

    Digital pulse shape analysis (dPSA) has been used with a Cuttler-Shalev type (3)He ionization chamber to measure the fast-neutron spectra of a deuterium-deuterium electronic neutron generator, a bare (252)Cf spontaneous fission neutron source, and of the transmitted fast neutron spectra of a (252)Cf source attenuated by water, graphite, liquid nitrogen, and magnesium. Rise-time dPSA has been employed using the common approach for analyzing n +(3)He→(1)H+(3)H ionization events and improved to account for wall-effect and pile-up events, increasing the fidelity of these measurements. Simulations have been performed of the different experimental arrangements and compared with the measurements, demonstrating general agreement between the dPSA-processed fast-neutron spectra and predictions. The fast-neutron resonance features of the attenuation cross sections of the attenuating materials are clearly visible within the resolution limits of the electronics used for the measurements, and the potential applications of high-resolution fast-neutron spectrometry for nuclear nonproliferation and safeguards measurements are discussed.

  8. Neutron noise measurements at the Delphi subcritical assembly

    SciTech Connect

    Szieberth, M.; Klujber, G.; Kloosterman, J. L.; De Haas, D.

    2012-07-01

    The paper presents the results and evaluations of a comprehensive set of neutron noise measurements on the Delphi subcritical assembly of the Delft Univ. of Technology. The measurements investigated the effect of different source distributions (inherent spontaneous fission and {sup 252}Cf) and the position of the detectors applied (both radially and vertically). The evaluation of the measured data has been performed by the variance-to-mean ratio (VTMR, Feynman-{alpha}), the autocorrelation (ACF, Rossi-{alpha}) and the cross-correlation (CCF) methods. The values obtained for the prompt decay constant show a strong bias, which depends both on the detector position and on the source distribution. This is due to the presence of higher modes in the system. It has been observed that the {alpha} value fitted is higher when the detector is close to the boundary of the core or to the {sup 252}Cf point-source. The higher alpha-modes have also been observed by fitting functions describing two alpha-modes. The successful set of measurement also provides a good basis for further theoretical investigations including the Monte Carlo simulation of the noise measurements and the calculation of the alpha-modes in the Delphi subcritical assembly. (authors)

  9. Facilitating Precision Mass Measurements at CARIBU

    NASA Astrophysics Data System (ADS)

    Lascar, Daniel; van Schelt, Jon; Savard, Guy; Segel, Ralph; Clark, Jason; Sharma, Kumar; Caldwell, Shane; Gang, Li; Sternberg, Matthew; Greene, John; Levand, Anthony; Zabransky, Bruce

    2011-10-01

    The Canadian Penning Trap Mass Spectrometer (CPT) has begun a campaign of precision mass measurements of neutron-rich nuclei produced via spontaneous fission of 252Cf as part of the CAlifornium Rare Isotope Breeder Upgrade (CARIBU) to the ATLAS facility at Argonne National Laboratory. As of the time of submission of this abstract, we have measured neutron rich isotopes of Cs, I, Te, Sb, and Sn. CARIBU is currently running with a 60 mCi source of 252Cf which will be upgraded to a 1 Ci source in the future. In order to make this campaign possible, several upgrades to the CARIBU and CPT system were required including a new Radio Frequency Quadrupole (RFQ) ion buncher to CARIBU's low energy beamline, cryogenic cooling of the RFQ Paul trap below the CPT, and an electrostatic elevator to allow for transport of ion bunches from a 50 kV platform to the CPT system's 2 kV beamline. Construction and commissioning of the buncher and modified Paul Trap will be discussed as well as their impact on the measurements in this campaign. Support from U.S. DOE, Nucl Phys Div and NSERC Canada.

  10. Spontaneous pneumothorax during pregnancy.

    PubMed

    Gorospe, Luis; Puente, Susana; Madrid, Carmen; Novo, Susana; Gil-Alonso, José L; Guntiñas, Alicia

    2002-05-01

    Spontaneous pneumothorax complicating pregnancy is rare. Only 41 cases have been previously published. We describe a case of spontaneous pneumothorax successfully treated with tube thoracostomy during the 38th week of pregnancy. Under epidural anesthesia, the patient had vaginal delivery of a healthy male infant 36 hours after tube thoracostomy.

  11. Novel calibration for LA-ICP-MS-based fission-track thermochronology

    NASA Astrophysics Data System (ADS)

    Soares, C. J.; Guedes, S.; Hadler, J. C.; Mertz-Kraus, R.; Zack, T.; Iunes, P. J.

    2014-01-01

    We present a novel age-equation calibration for fission-track age determinations by laser ablation inductively coupled plasma mass spectrometry. This new calibration incorporates the efficiency factor of an internal surface, [ ηq]is, which is obtained by measuring the projected fission-track length, allowing the determination of FT ages directly using the recommended spontaneous fission decay constant. Also, the uranium concentrations in apatite samples are determined using a Durango (Dur-2, 7.44 μg/g U) crystal and a Mud Tank (MT-7, 6.88 μg/g U) crystal as uranium reference materials. The use of matrix-matched reference materials allows a reduction in the uncertainty of the uranium measurements to those related to counting statistics, which are ca. 1 % taking into account that no extra source of uncertainty has to be considered. The equations as well as the matrix-matched reference materials are evaluated using well-dated samples from Durango, Fish Canyon Tuff, and Limberg as unknown samples. The results compare well with their respective published ages determined through other dating methods. Additionally, the results agree with traditional fission-track ages using both the zeta approach and the absolute approach, suggesting that the calibration presented in this work can be robustly applied in geological context. Furthermore, considering that fission-track ages can be determined without an age standard sample, the fission-track thermochronology approach presented here is assumed to be a valuable dating tool.

  12. Development of a thin scintillation films fission-fragment detector and a novel neutron source

    SciTech Connect

    Rusev, Gencho Yordanov; Jandel, Marian; Baramsai, Bayarbadrakh; Bond, Evelyn M.; Bredeweg, Todd Allen; Couture, Aaron Joseph; Daum, Jaimie Kay; Favalli, Andrea; Ianakiev, Kiril Dimitrov; Iliev, Metodi L.; Mosby, Shea Morgan; Roman, Audrey Rae; Springs, Rebecca Kristien; Ullmann, John Leonard; Walker, Carrie Lynn

    2015-08-26

    Here, investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flight spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

  13. Fission track analysis, rift shoulder uplift, and tectonic modeling of the Norwegian Continental Margin

    SciTech Connect

    Andriessen, P.; Van Der Beek, P.; Cloetingh, S.; Rohrman, M. )

    1993-09-01

    Apatite fission track analysis from southern Norway and Sweden, across the Permian Carboniferous Oslo rift, are presented and discussed in relation to different rifting scenarios. Vertical and horizontal apatite fission tack profiles in middle and southern Norway unravel the post-Carboniferous history of the Fennoscandian shield. Fission track apatite ages range from 240 Ma in the south to 160 Ma in the north, and according to spontaneous fission track length measurements, they must be interpreted as mixed ages, indicating minor amounts of Paleozoic-Mesozoic sedimentary cover. Apatite fission track length and age modeling suggest rapid cooling and uplift in the Tertiary for the southernmost part of Norway, suggesting a differential uplift of the basement. the obtained data are important for the reconstruction of burial and thermal histories of Cenozoic sedimentary basins of the Norwegian continental margin in the northern North Sea, where diverse rifting events, intraplate stress regimes, and inversion tectonics are involved. Fission track analysis puts constraints on tectonic modeling of uplift of rift flanks and the Norwegian continental margin and yields information for these assessment of hydrocarbon potentials of the sedimentary basins.

  14. Velocity fluctuations of fission fragments

    NASA Astrophysics Data System (ADS)

    Llanes-Estrada, Felipe J.; Carmona, Belén Martínez; Martínez, Jose L. Muñoz

    2016-02-01

    We propose event by event velocity fluctuations of nuclear fission fragments as an additional interesting observable that gives access to the nuclear temperature in an independent way from spectral measurements and relates the diffusion and friction coefficients for the relative fragment coordinate in Kramers-like models (in which some aspects of fission can be understood as the diffusion of a collective variable through a potential barrier). We point out that neutron emission by the heavy fragments can be treated in effective theory if corrections to the velocity distribution are needed.

  15. PRODUCING ENERGY AND RADIOACTIVE FISSION PRODUCTS

    DOEpatents

    Segre, E.; Kennedy, J.W.; Seaborg, G.T.

    1959-10-13

    This patent broadly discloses the production of plutonium by the neutron bombardment of uranium to produce neptunium which decays to plutonium, and the fissionability of plutonium by neutrons, both fast and thermal, to produce energy and fission products.

  16. Neutronics for critical fission reactors and subcritical fission in hybrids

    NASA Astrophysics Data System (ADS)

    Salvatores, Massimo

    2012-06-01

    The requirements of future innovative nuclear fuel cycles will focus on safety, sustainability and radioactive waste minimization. Critical fast neutron reactors and sub-critical, external source driven systems (accelerator driven and fusion-fission hybrids) have a potential role to meet these requirements in view of their physics characteristics. This paper provides a short introduction to these features.

  17. Neutronics for critical fission reactors and subcritical fission in hybrids

    SciTech Connect

    Salvatores, Massimo

    2012-06-19

    The requirements of future innovative nuclear fuel cycles will focus on safety, sustainability and radioactive waste minimization. Critical fast neutron reactors and sub-critical, external source driven systems (accelerator driven and fusion-fission hybrids) have a potential role to meet these requirements in view of their physics characteristics. This paper provides a short introduction to these features.

  18. An alternative calibration method for counting P-32 reactor monitors

    SciTech Connect

    Quirk, T.J.; Vehar, D.W.

    2011-07-01

    Radioactivation of sulfur is a common technique used to measure fast neutron fluences in test and research reactors. Elemental sulfur can be pressed into pellets and used as monitors. The {sup 32}S(n, p) {sup 32}P reaction has a practical threshold of about 3 MeV and its cross section and associated uncertainties are well characterized [1]. The product {sup 32P} emits a beta particle with a maximum energy of 1710 keV [2]. This energetic beta particle allows pellets to be counted intact. ASTM Standard Test Method for Measuring Reaction Rates and Fast-Neutron Fluences by Radioactivation of Sulfur-32 (E265) [3] details a method of calibration for counting systems and subsequent analysis of results. This method requires irradiation of sulfur monitors in a fast-neutron field whose spectrum and intensity are well known. The resultant decay-corrected count rate is then correlated to the known fast neutron fluence. The Radiation Metrology Laboratory (RML) at Sandia has traditionally performed calibration irradiations of sulfur pellets using the {sup 252}Cf spontaneous fission neutron source at the National Inst. of Standards and Technology (NIST) [4] as a transfer standard. However, decay has reduced the intensity of NIST's source; thus lowering the practical upper limits of available fluence. As of May 2010, neutron emission rates have decayed to approximately 3 e8 n/s. In practice, this degradation of capabilities precludes calibrations at the highest fluence levels produced at test reactors and limits the useful range of count rates that can be measured. Furthermore, the reduced availability of replacement {sup 252}Cf threatens the long-term viability of the NIST {sup 252}Cf facility for sulfur pellet calibrations. In lieu of correlating count rate to neutron fluence in a reference field the total quantity of {sup 32}P produced in a pellet can be determined by absolute counting methods. This offers an attractive alternative to extended {sup 252}Cf exposures because it

  19. Process for treating fission waste. [Patent application

    DOEpatents

    Rohrmann, C.A.; Wick, O.J.

    1981-11-17

    A method is described for the treatment of fission waste. A glass forming agent, a metal oxide, and a reducing agent are mixed with the fission waste and the mixture is heated. After melting, the mixture separates into a glass phase and a metal phase. The glass phase may be used to safely store the fission waste, while the metal phase contains noble metals recovered from the fission waste.

  20. The role of off-line mass spectrometry in nuclear fission.

    PubMed

    De Laeter, J R

    1996-01-01

    The role of mass spectrometry in nuclear fission has been invaluable since 1940, when A. O. C. Nier separated microgram quantities of (235) U from (238) U, using a gas source mass spectrometer. This experiment enabled the fissionable nature of (235) U to be established. During the Manhattan Project, the mass spectrometer was used to measure the isotope abundances of uranium after processing in various separation systems, in monitoring the composition of the gaseous products in the Oak Ridge Diffusion Plant, and as a helium leak detector. Following the construction of the first reactor at the University of Chicago, it was necessary to unravel the nuclear systematics of the various fission products produced in the fission process. Off-line mass spectrometry was able to identify stable and long-lived isotopes produced in fission, but more importantly, was used in numerous studies of the distribution of mass of the cumulative fission yields. Improvements in sensitivity enabled off-line mass spectrometric studies to identify fine structure in the mass-yield curve and, hence, demonstrate the importance of shell structure in nuclear fission. Solid-source mass spectrometry was also able to measure the cumulative fission yields in the valley of symmetry in the mass-yield curve, and enabled spontaneous fission yields to be quantified. Apart from the accurate measurement of abundances, the stable isotope mass spectrometric technique has been invaluable in establishing absolute cumulative fission yields for many isotopes making up the mass-yield distribution curve for a variety of fissile nuclides. Extensive mass spectrometric studies of noble gases in primitive meteorites revealed the presence of fission products from the now extinct nuclide (244) Pu, and have eliminated the possibility of fission products from a super-heavy nuclide contributing to isotopic anomalies in meteoritic material. Numerous mass spectrometric studies of the isotopic and elemental abundances of

  1. Etching fission tracks in zircons

    USGS Publications Warehouse

    Naeser, C.W.

    1969-01-01

    A new technique has been developed whereby fission tracks can be etched in zircon with a solution of sodium hydroxide at 220??C. Etching time varied between 15 minutes and 5 hours. Colored zircon required less etching time than the colorless varieties.

  2. Space Fission System Test Effectiveness

    SciTech Connect

    Houts, Mike; Schmidt, Glen L.; Van Dyke, Melissa; Godfroy, Tom; Martin, James; Bragg-Sitton, Shannon; Dickens, Ricky; Salvail, Pat; Harper, Roger

    2004-02-04

    Space fission technology has the potential to enable rapid access to any point in the solar system. If fission propulsion systems are to be developed to their full potential, however, near-term customers need to be identified and initial fission systems successfully developed, launched, and utilized. One key to successful utilization is to develop reactor designs that are highly testable. Testable reactor designs have a much higher probability of being successfully converted from paper concepts to working space hardware than do designs which are difficult or impossible to realistically test. ''Test Effectiveness'' is one measure of the ability to realistically test a space reactor system. The objective of this paper is to discuss test effectiveness as applied to the design, development, flight qualification, and acceptance testing of space fission systems. The ability to perform highly effective testing would be particularly important to the success of any near-term mission, such as NASA's Jupiter Icy Moons Orbiter, the first mission under study within NASA's Project Prometheus, the Nuclear Systems Program.

  3. A practical method of estimating standard error of age in the fission track dating method

    USGS Publications Warehouse

    Johnson, N.M.; McGee, V.E.; Naeser, C.W.

    1979-01-01

    A first-order approximation formula for the propagation of error in the fission track age equation is given by PA = C[P2s+P2i+P2??-2rPsPi] 1 2, where PA, Ps, Pi and P?? are the percentage error of age, of spontaneous track density, of induced track density, and of neutron dose, respectively, and C is a constant. The correlation, r, between spontaneous are induced track densities is a crucial element in the error analysis, acting generally to improve the standard error of age. In addition, the correlation parameter r is instrumental is specifying the level of neutron dose, a controlled variable, which will minimize the standard error of age. The results from the approximation equation agree closely with the results from an independent statistical model for the propagation of errors in the fission-track dating method. ?? 1979.

  4. DETECTORS AND EXPERIMENTAL METHODS: Equivalent properties of single event burnout induced by different sources

    NASA Astrophysics Data System (ADS)

    Yang, Shi-Yu; Cao, Zhou; Da, Dao-An; Xue, Yu-Xiong

    2009-05-01

    The experimental results of single event burnout induced by heavy ions and 252Cf fission fragments in power MOSFET devices have been investigated. It is concluded that the characteristics of single event burnout induced by 252Cf fission fragments is consistent to that in heavy ions. The power MOSFET in the “turn-off" state is more susceptible to single event burnout than it is in the “turn-on" state. The thresholds of the drain-source voltage for single event burnout induced by 173 MeV bromine ions and 252Cf fission fragments are close to each other, and the burnout cross section is sensitive to variation of the drain-source voltage above the threshold of single event burnout. In addition, the current waveforms of single event burnouts induced by different sources are similar. Different power MOSFET devices may have different probabilities for the occurrence of single event burnout.

  5. Two neutron correlations in photo-fission

    NASA Astrophysics Data System (ADS)

    Dale, D. S.; Kosinov, O.; Forest, T.; Burggraf, J.; Stave, S.; Warren, G.; Starovoitova, V.

    2016-09-01

    A large body of experimental work has established the strong kinematical correlation between fission fragments and fission neutrons. Here, we report on the progress of investigations of the potential for strong two neutron correlations arising from the nearly back-to-back nature of the two fission fragments that emit these neutrons in the photo-fission process. In initial measurements, a pulsed electron linear accelerator was used to generate bremsstrahlung photons that impinged upon an actinide target, and the energy and opening angle distributions of coincident neutrons were measured using a large acceptance neutron detector array. A planned comprehensive set of measurements of two neutron correlations in the photo-fission of actinides is expected to shed light on several fundamental aspects of the fission process including the multiplicity distributions associated with the light and heavy fission fragments, the nuclear temperatures of the fission fragments, and the mass distribution of the fission fragments as a function of energy released. In addition to these measurements providing important nuclear data, the unique kinematics of fission and the resulting two neutron correlations have the potential to be the basis for a new tool to detect fissionable materials. A key technical challenge of this program arises from the need to perform coincidence measurements with a low duty factor, pulsed electron accelerator. This has motivated the construction of a large acceptance neutron detector array, and the development of data analysis techniques to directly measure uncorrelated two neutron backgrounds.

  6. Space Fission Propulsion System Development Status

    NASA Technical Reports Server (NTRS)

    Houts, Mike; VanDyke, Melissa; Godfroy, Tom; Pedersen, Kevin; Martin, James; Dickens, Ricky; Williams, Eric; Harper, Roger; Salvail, Pat; Hrbud, Ivana; Rodgers, Stephen L. (Technical Monitor)

    2001-01-01

    The world's first man-made self-sustaining fission reaction was achieved in 1942. Since then fission has been used to propel submarines, generate tremendous amounts of electricity, produce medical isotopes, and provide numerous other benefits to society. Fission systems operate independently of solar proximity or orientation, and are thus well suited for deep spare or planetary surface missions. In addition, the fuel for fission systems (enriched uranium) is virtually non-radioactive. The primary safety issue with fission systems is avoiding inadvertent system start - addressing this issue through proper system design is straightforward. Despite the relative simplicity and tremendous potential of space fission systems, the development and utilization of these systems has proven elusive. The first use of fission technology in space occurred 3 April 1965 with the US launch of the SNAP-10A reactor. There have been no additional US uses of space fission system. While space fission system were used extensively by the former Soviet Union, their application was limited to earth-orbital missions. Early space fission systems must be safely and affordably utilized if Ae are to reap the benefits of advanced space fission systems.

  7. Spontaneous combustion of hydrogen

    NASA Technical Reports Server (NTRS)

    Nusselt, Wilhelm; Pothmann, PH

    1923-01-01

    It is shown by the author's experiments that hydrogen which escapes to the atmosphere through openings in the system may burn spontaneously if it contains dust. Purely thermal reasoning can not account for the combustion. It seems to be rather an electrical ignition. In order to determine whether the cause of the spontaneous ignition was thermo-chemical, thermo-mechanical, or thermo-electrical, the experiments in this paper were performed.

  8. Spontaneous cholecystocutaneous abscess.

    PubMed

    Metsemakers, W J; Quanten, I; Vanhoenacker, F; Spiessens, T

    2010-01-01

    Spontaneous cholecystocutaneous abscesses or fistulae are rare complications of neglected biliary calculous disease which have become extremely rare during the last decades. We report a case of spontaneous cholecystocutaneous abscess in a 69-year-old male who presented with a mass in the right subcostal region.The diagnosis was made by CT scan with multiplanar reformating. Treatment consisted of incision and drainage of the abdominal wall abscess followed by cholecystectomy in a one-stage protocol.

  9. Experimental study of the three-component structure of mass-energy distributions of fission fragments of nuclei in the vicinity of Pb

    SciTech Connect

    Gruzintsev, E.N.; Itkis, M.G.; Kotlov, Y.V.; Okolovich, V.N.; Rusanov, A.Y.; Smirenkin, G.N.

    1988-05-01

    Measurements and a regression analysis of mass-energy distributions of fission fragments of the nuclei /sup 213/At, /sup 210/Po, and /sup 205/Bi were carried out, demonstrating a three-component structure in the kinetic energy spectra of fragments. The nature of this phenomenon is discussed, as well as its similarity to the recently observed bimodal spontaneous fission of nuclei in the vicinity of Fm.

  10. Plutonium-244 fission tracks - Evidence in a lunar rock 3.95 billion years old.

    NASA Technical Reports Server (NTRS)

    Hutcheon, I. D.; Price, P. B.

    1972-01-01

    Tracks attributed to the spontaneous fission of plutonium-244 and of uranium-238 were detected in a large whitlockite crystal in the lunar breccia 14321 from the Fra Mauro formation. For a track-retention age of 3.95 b.y., the number of plutonium tracks relative to the number of uranium tracks is 0.51 plus or minus 0.15, provided that the rock was not heavily neutron-irradiated 3.95 b.y. ago.

  11. Collective Inertia and Fission Barriers Within the Skyrme-Hartree-Fock Theory

    SciTech Connect

    Baran, A.; Staszczak, A.; Dobaczewski, J.; Nazarewicz, Witold

    2007-01-01

    Spontaneous fission barriers, quadrupole inertia tensor, and zero-point quadrupole correlation energy are calculated for 252,256,258Fm in the framework of the self-consistent Skyrme-Hartree-Fock+BCS theory. Two ways of computing collective inertia are employed: the Gaussian Overlap Approximation to the Generator Coordinate Method and cranking ansatz. The Skyrme results are compared with those of the Gogny-Hartree-Fock-Bogoliubov model.

  12. Space Fission Propulsion System Development Status

    NASA Technical Reports Server (NTRS)

    Houts, M.; Van Dyke, M. K.; Godfroy, T. J.; Pedersen, K. W.; Martin, J. J.; Dickens, R.; Williams, E.; Harper, R.; Salvail, P.; Hrbud, I.

    2001-01-01

    The world's first man-made self-sustaining fission reaction was achieved in 1942. Since then fission has been used to propel submarines, generate tremendous amounts of electricity, produce medical isotopes, and provide numerous other benefits to society. Fission systems operate independently of solar proximity or orientation, and are thus well suited for deep space or planetary surface missions. In addition, the fuel for fission systems (enriched uranium) is virtually non-radioactive. The primary safety issue with fission systems is avoiding inadvertent system start. Addressing this issue through proper system design is straight-forward. Despite the relative simplicity and tremendous potential of space fission systems, the development and utilization of these systems has proven elusive. The first use of fission technology in space occurred 3 April 1965 with the US launch of the SNAP-10A reactor. There have been no additional US uses of space fission systems. While space fission systems were used extensively by the former Soviet Union, their application was limited to earth-orbital missions. Early space fission systems must be safely and affordably utilized if we are to reap the benefits of advanced space fission systems. NASA's Marshall Space Flight Center, working with Los Alamos National Laboratory (LANL), Sandia National Laboratories, and others, has conducted preliminary research related to a Safe Affordable Fission Engine (SAFE). An unfueled core has been fabricated by LANL, and resistance heaters used to verify predicted core thermal performance by closely mimicking heat from fission. The core is designed to use only established nuclear technology and be highly testable. In FY01 an energy conversion system and thruster will be coupled to the core, resulting in an 'end-to-end' nuclear electric propulsion demonstrator being tested using resistance heaters to closely mimic heat from fission. Results of the SAFE test program will be presented. The applicability

  13. Fission and Properties of Neutron-Rich Nuclei

    NASA Astrophysics Data System (ADS)

    Hamilton, Joseph H.; Ramayya, A. V.; Carter, H. K.

    2008-08-01

    . Fission-fragment spectroscopy with STEFF / A. G. Smith ... [et al.]. Gamma ray multiplicity of [symbol]Cf spontaneous fission using LiBerACE / D. L. Bleuel ... [et al.]. Excitation energy dependence of fragment mass and total kinetic energy distributions in proton-induced fission of light actinides / I. Nishinaka ... [et al.]. A dynamical calculation of multi-modal nuclear fission / T. Wada and T. Asano. Structure of fission potential energy surfaces in ten-dimensional spaces / V. V. Pashkevich, Y. K Pyatkov and A. V. Unzhakova. A possible enhancement of nuclear fission in scattering with low energy charged particles / V. Gudkov. Dynamical multi-break processes in the [symbol]Sn + [symbol]Ni system at 35 MeV/Nucleon / M. Papa and ISOSPIN-RE VERSE collaboration -- New experimental techniques. MTOF - a high resolution isobar separator for studies of exotic decays / A. Piechaczek ... [et al.]. Development of ORRUBA: a silicon array for the measurement of transfer reactions in inverse kinematics / S. D. Pain ... [et al.]. Indian national gamma array: present & future / R. K. Bhowmik. Absolute intensities of [symbol] rays emitted in the decay of [symbol]U / H. C. Griffin -- Superheavy elements theory and experiments / M. G. Itkis ... [et al.]. Study of superheavy elements at SHIP / S. Hofinann. Heaviest nuclei from [symbol]Ca-induced reactions / Yu. Ts. Oaanessian. Superheavy nuclei and giant nuclear systems / W. Greiner and V. Zagrebaev. Fission approach to alpha-decay of superheavy nuclei / D.N. Poenaru and W. Greiner. Superheavy elements in the Magic Islands / C. Samanta. Relativistic mean field studies of superheavy nuclei / A. V. Afanas jev. Understanding the synthesis of the heaviest nuclei / W. Loveland -- Mass measurements and g-factors. G factor measurements in neutron-rich [symbol]Cf fission fragments, measured using the gammasphere array / R. Orlandi ... [et al.]. Technique for measuring angular correlations and g-factors in neutron rich nuclei produced by the

  14. Bright fission: singlet fission into a pair of emitting states.

    PubMed

    Casanova, David

    2015-06-01

    This paper reintroduces and explores the generation of two bright states from a single photon via a singlet fission mechanism in organic materials. This particular photophysical process is labeled here as bright fission (BF). The central part of the study is devoted to set the theoretical foundations of BF by discussing possible electronic mechanisms, the role of different excited states with various physical nature, the presence of competing deactivation channels, and the possible requirements for the BF viability. In a second part, some of the properties related to BF are computationally explored in anthracene. The analysis of computed high-lying excited states identifies several optical transitions as good candidates to trigger BF in anthracene. The approximation of excitonic couplings of these high energy levels to other electronic states within the same energy range suggests possible paths to populate electronic configurations potentially able to split in two independent spin singlets, i.e. singlet-singlet states. The study also explores the electronic structure of the energetically lowest singlet-singlet states in anthracene dimers and discusses the presence of charge transfer configurations and their relation to the singlet-singlet manifold. The computational results suggest fast relaxation to the lowest singlet-singlet state, from which the excitonic fission may occur. All in all, the present work aims at motivating to pursue further efforts in the study of the BF process in organic materials.

  15. Fission Properties for R-Process Nuclei

    SciTech Connect

    Erler, J.

    2012-01-01

    We present a systematics of fission barriers and fission lifetimes for the whole landscape of superheavy elements (SHE), i.e., nuclei with Z 100. The fission lifetimes are also compared with the -decay half-lives. The survey is based on a self-consistent description in terms of the Skyrme-Hartree-Fock (SHF) approach. Results for various different SHF parametrizations are compared to explore the robustness of the predictions. The fission path is computed by quadrupole constrained SHF. The computation of fission lifetimes takes care of the crucial ingredients of the large-amplitude collective dynamics along the fission path, as self-consistent collective mass and proper quantum corrections. We discuss the different topologies of fission landscapes which occur in the realm of SHE (symmetric versus asymmetric fission, regions of triaxial fission, bimodal fission, and the impact of asymmetric ground states). The explored region is extended deep into the regime of very neutron-rich isotopes as they are expected to be produced in the astrophysical r process.

  16. Technical Application of Nuclear Fission

    NASA Astrophysics Data System (ADS)

    Denschlag, J. O.

    The chapter is devoted to the practical application of the fission process, mainly in nuclear reactors. After a historical discussion covering the natural reactors at Oklo and the first attempts to build artificial reactors, the fundamental principles of chain reactions are discussed. In this context chain reactions with fast and thermal neutrons are covered as well as the process of neutron moderation. Criticality concepts (fission factor η, criticality factor k) are discussed as well as reactor kinetics and the role of delayed neutrons. Examples of specific nuclear reactor types are presented briefly: research reactors (TRIGA and ILL High Flux Reactor), and some reactor types used to drive nuclear power stations (pressurized water reactor [PWR], boiling water reactor [BWR], Reaktor Bolshoi Moshchnosti Kanalny [RBMK], fast breeder reactor [FBR]). The new concept of the accelerator-driven systems (ADS) is presented. The principle of fission weapons is outlined. Finally, the nuclear fuel cycle is briefly covered from mining, chemical isolation of the fuel and preparation of the fuel elements to reprocessing the spent fuel and conditioning for deposit in a final repository.

  17. Triaxial and Triaxial Softness in Neutron Rich ru and pd Nuclei

    NASA Astrophysics Data System (ADS)

    Luo, Y. X.; Hamilton, J. H.; Ramaya, A. V.; Hwang, J. K.; Liu, S. H.; Rasmussen, J. O.; Frauendorf, S.; Ter-Akopian, G. M.; Daniel, A. V.; Oganessian, Yu. Ts.; Zhu, S. J.

    2013-06-01

    The level structures of 108,110,112Ru (Z=44) and 112,114,115,116,117,118Pd (Z=46) have been significantly expanded through studies of prompt γ-γ-γ coincidences observed with Gammasphere following the spontaneous fission of 252Cf. The softness to triaxiality perturbs the band structures of 108Ru and even-N Pd isotopes. Two sets of odd-parity bands are identified in 112,114,116Pd similar to but different from those in 110,112Ru. These differences can be accounted for by interferences of the chiral doubling and softness to triaxiality. Also in 112Ru, evidence for wobbling motion is found in the behavior of the γ vibrational band. Similar evidence for wobbling motion is found in 114Pd, the N = 68 isotone of 112Ru.

  18. Proposed s =±1 octupole bands in 140Xe

    NASA Astrophysics Data System (ADS)

    Huang, Y.; Zhu, S. J.; Hamilton, J. H.; Wang, E. H.; Ramayya, A. V.; Xiao, Z. G.; Li, H. J.; Luo, Y. X.; Rasmussen, J. O.; Ter-Akopian, G. M.; Oganessian, Yu. Ts.

    2016-06-01

    Level structures of neutron-rich 140Xe nucleus have been reinvestigated by using a triple γ coincidence study from the spontaneous fission of 252Cf. Several new levels and transitions are identified. The previously observed s =+1 octupole band structure is confirmed and expanded. Another set of the Δ I =2 positive and negative parity bands connected by strong E 1 transitions is proposed as the s =-1 octupole band structure. Thus, the s =±1 doublet octupole bands are completed in 140Xe. The experimental B (E 1 )/B (E 2 ) branching ratios indicate that the octupole correlations in 140Xe are weak. The other characteristics of the s =±1 octupole bands have been discussed.

  19. Evidence for Chiral Doublet Bands in 110,112Ru

    NASA Astrophysics Data System (ADS)

    Luo, Y. X.; Zhu, S. J.; Hamilton, J. H.; Rasmussen, J. O.; Ramayya, A. V.; Goodin, C.; Li, K.; Hwang, J. K.; Che, X. L.; Jang, Z.; Frauendorf, S.; Dimitrov, V.; Zhang, Jing-Ye; Stefanescu, I.; Gelberg, A.; Ter-Akopian, G. M.; Daniel, A. V.; Stoyer, M. A.; Donangelo, R.; Cole, J. D.; Stone, N. J.

    2008-08-01

    From γ-γ-γ coincidence studies of prompt γ rays in the spontaneous fission from 252Cf with Gammasphere, two sets of ΔI = 1 doublet bands assigned odd-parities were identified in 108,110,112Ru. γ-γ (θ) angular correlation data were analyzed to assign multipolarities of the depopulating transitions and spins of the bandheads. The above assignments and the decay pattern of the levels uniquely support the odd-parity assignment of the doublet bands. By checking characteristic conditions for generating chiral symmetry breaking and the fingerprints as expected for observations of chiral doublet bands in the nuclei, and based on the Tilted Axis Cranking calculations, the Δ I = 1 odd-parity doublet bands identified in 110,112Ru are assigned zero and one phonon chiral vibration bands built on υ h11/2 × (d5/2g7/2)-1 configuration.

  20. High-spin states in {sup 91,92,93}Rb and {sup 155,156}Pm

    SciTech Connect

    Hwang, J. K.; Ramayya, A. V.; Hamilton, J. H.; Liu, S. H.; Li, K.; Crowell, H. L.; Goodin, C.; Luo, Y. X.; Rasmussen, J. O.; Zhu, S. J.

    2009-09-15

    The excited states of the neutron-rich nuclei {sup 155,156}Pm and {sup 91,92,93}Rb were studied from the spontaneous fission of {sup 252}Cf. The {gamma}-{gamma}-{gamma} and x(Pm)-{gamma}-{gamma} triple coincidence relations were applied to identify the {gamma} transitions. Fourteen, six, three, twelve, and twelve new {gamma} transitions from high-spin states were observed in {sup 155,156}Pm, {sup 91,92}Rb, and {sup 93}Rb (first levels), respectively. The {pi}5/2[532] rotational band in {sup 155}Pm was extended up to 23/2{sup -}. The {pi}g{sub 9/2} particle states and {pi}f{sub 5/2} particle states in {sup 91,93}Rb weakly coupled to {sup 90,92}Kr, respectively, are reported.

  1. Identification of a quasiparticle band in very neutron-rich {sup 104}Zr

    SciTech Connect

    Yeoh, E. Y.; Wang, J. G.; Ding, H. B.; Gu, L.; Xu, Q.; Xiao, Z. G.; Zhu, S. J.; Hamilton, J. H.; Ramayya, A. V.; Hwang, J. K.; Liu, S. H.; Liu, Y. X.; Sun, Y.; Luo, Y. X.; Rasmussen, J. O.; Lee, I. Y.

    2010-08-15

    The high spin levels of a very neutron-rich {sup 104}Zr nucleus have been reinvestigated by measuring the prompt {gamma} rays in the spontaneous fission of {sup 252}Cf. The ground-state band has been confirmed. A new sideband has been identified with a band-head energy at 1928.7 keV. The projected shell model is employed to investigate the band structure of {sup 104}Zr. The results of calculated levels are in good agreement with the experimental data, and suggest that the new band in {sup 104}Zr may be based on the neutron {nu}5/2{sup -}[532] x {nu}3/2{sup +}[411] configuration.

  2. Commissioning a Tape Transport System for Decay Studies and Beam Diagnostics at CARIBU

    NASA Astrophysics Data System (ADS)

    Bertone, P. F.; Digiovine, B.; Lister, C. J.; Teh, K.; Kondev, F. G.; Nair, C.; Chowdhury, P.; Deo, A. Y.; Lakshmi, S.

    2011-10-01

    The CAlifornium Rare Isotope Breeder Upgrade (CARIBU) to the ATLAS facility at Argonne utilizes the spontaneous fission of 252 Cf for producing neutron-rich radioactive nuclei. CARIBU will be used for a wide variety of experiments, involving both reaccelerated and stopped beams, in nuclear structure, nuclear astrophysics and applications. Many of these experiments will require a means of transporting radioactivity to and from detector counting stations for the purpose of assaying beam content, measuring half-lives, β- γ spectroscopy and determining Gamow-Teller strength distributions. We have commissioned the first of several tape transport systems that will perform these functions. An overview of the design and deployment of the system will be given along with preliminary test results. Supported by the U.S. DOE Office of Nuclear Physics DE-AC02-06CH11357.

  3. Possible excited deformed rotational bands in {sup 82}Ge

    SciTech Connect

    Hwang, J. K.; Hamilton, J. H.; Ramayya, A. V.; Brewer, N. T.; Luo, Y. X.; Rasmussen, J. O.; Zhu, S. J.

    2011-08-15

    Excited states of neutron-rich nucleus {sup 82}Ge were studied from the spontaneous fission of {sup 252}Cf. Eleven new transitions and seven new levels in {sup 82}Ge were identified by using X(Dy)-{gamma}-{gamma} and {gamma}-{gamma}-{gamma} triple coincidences. Possible excited deformed rotational bands are observed, for the first time, in this nuclear region. Coexistence of the spherical ground and deformed excited shapes is proposed in {sup 82}Ge. These deformed rotational bands can be formed by two-particle, two-hole excitations with the 0{sup +} pairing energy states of the {nu}9/2[404]{sup -2} x 1/2[431]{sup 2} configuration across the N=50 closed shell.

  4. High-spin level structure of {sup 115}Rh: Evolution of triaxiality in odd-even Rh isotopes

    SciTech Connect

    Liu, S. H.; Gelberg, A.; Gu, L.; Yeoh, E. Y.; Zhu, S. J.; Luo, Y. X.; Rasmussen, J. O.; Ma, W. C.; Daniel, A. V.; Oganessian, Yu. Ts.; Ter-Akopian, G. M.

    2011-07-15

    High-spin excited states in the neutron-rich nucleus {sup 115}Rh have been identified for the first time by studying prompt {gamma} rays from the spontaneous fission of {sup 252}Cf with the Gammasphere detector array. A new yrast band and a sideband are built in {sup 115}Rh. This level scheme is proposed to be built on the 7/2{sup +} ground state. The existence of a large signature splitting and an yrare band in {sup 115}Rh shows typical features of a triaxially deformed nucleus. The rigid triaxial rotor plus particle model is used to interpret the level structure of {sup 115}Rh. The level energies, the {gamma} branching ratios, the large signature splitting in the yrast band, and the inverted signature splitting in the yrare band in {sup 115}Rh are reproduced very well. Strong K mixing occurs in {sup 115}Rh at high spin.

  5. New Band Structures in Aapprox110 Neutron-Rich Nuclei

    SciTech Connect

    Zhu, S. J.; Wang, J. G.; Ding, H. B.; Gu, L.; Xu, Q.; Yeoh, E. Y.; Xiao, Z. G.; Hamilton, J. H.; Ramayya, A. V.; Hwang, J. K.; Liu, S. H.; Li, K.; Luo, Y. X.; Rasmussen, J. O.; Lee, I. Y.; Qi, B.; Meng, J.

    2010-05-12

    The high spin states of neutron-rich nuclei in Aapprox110 region have been carefully investigated by measuring prompt gamma-gamma-gamma coincident measurements populated in the spontaneous fission of {sup 252}Cf with the Gammasphere detector array. Many new collective bands have been discovered. In this proceeding paper, we introduce some interesting new band structures recently observed by our cooperative groups, that is, the one-phonon- and two-phonon gamma-vibrational bands in odd-A {sup 103}Nb, {sup 105}Mo and {sup 107}Tc, the chiral doublet bands in even-even {sup 106}Mo, {sup 110}Ru and {sup 112}Ru, and the pseudospin partner bands with in {sup 108}Tc. The characteristics of these band structures have been discussed.

  6. Structure of the yrast band in the odd-odd deformed nucleus {sup 156}Pm

    SciTech Connect

    Sood, P. C.; Sai, K. Vijay; Gowrishankar, R.; Sainath, M.

    2011-05-15

    The six-level sequence deduced for the odd-odd nucleus {sup 156}Pm in the high-spin studies following spontaneous fission of {sup 252}Cf is shown to constitute the K{sup {pi}=}4{sup +} yrast band having the two-quasiparticle configuration {l_brace}p:5/2[532]+ n:3/2[521]{r_brace}. Spin parities I{sup {pi}=}4{sup +} through 9{sup +} are assigned to the earlier suggested six levels. The location and the decay {gamma}'s of the 10{sup +} level of this band are indicated. It is also pointed out that there are no {gamma} rays common to these postfission high-spin spectra and those seen in the {sup 156}Nd {beta}-decay studies.

  7. MODELING AND FISSION CROSS SECTIONS FOR AMERICIUM.

    SciTech Connect

    ROCHMAN, D.; HERMAN, M.; OBLOZINSKY, P.

    2005-05-01

    This is the final report of the work performed under the LANL contract on the modeling and fission cross section for americium isotopes (May 2004-June 2005). The purpose of the contract was to provide fission cross sections for americium isotopes with the nuclear reaction model code EMPIRE 2.19. The following work was performed: (1) Fission calculations capability suitable for americium was implemented to the EMPIRE-2.19 code. (2) Calculations of neutron-induced fission cross sections for {sup 239}Am to {sup 244g}Am were performed with EMPIRE-2.19 for energies up to 20 MeV. For the neutron-induced reaction of {sup 240}Am, fission cross sections were predicted and uncertainties were assessed. (3) Set of fission barrier heights for each americium isotopes was chosen so that the new calculations fit the experimental data and follow the systematics found in the literature.

  8. Spontaneous sarcomere dynamics

    NASA Astrophysics Data System (ADS)

    Günther, Stefan; Kruse, Karsten

    2010-12-01

    Sarcomeres are the basic force generating units of striated muscles and consist of an interdigitating arrangement of actin and myosin filaments. While muscle contraction is usually triggered by neural signals, which eventually set myosin motors into motion, isolated sarcomeres can oscillate spontaneously between a contracted and a relaxed state. We analyze a model for sarcomere dynamics, which is based on a force-dependent detachment rate of myosin from actin. Our numerical bifurcation analysis of the spontaneous sarcomere dynamics reveals notably Hopf bifurcations, canard explosions, and gluing bifurcations. We discuss possible implications for experiments.

  9. Comparative evaluation of solar, fission, fusion, and fossil energy resources. Part 2: Power from nuclear fission

    NASA Technical Reports Server (NTRS)

    Clement, J. D.

    1973-01-01

    Different types of nuclear fission reactors and fissionable materials are compared. Special emphasis is placed upon the environmental impact of such reactors. Graphs and charts comparing reactor facilities in the U. S. are presented.

  10. RECOVERY OF ALUMINUM FROM FISSION PRODUCTS

    DOEpatents

    Blanco, R.E.; Higgins, I.R.

    1962-11-20

    A method is given for recovertng aluminum values from aqueous solutions containing said values together with fission products. A mixture of Fe/sub 2/O/ sub 3/ and MnO/sub 2/ is added to a solution containing aluminum and fission products. The resulting aluminum-containing supernatant is then separated from the fission product-bearing metal oxide precipitate and is contacted with a cation exchange resin. The aluminum sorbed on the resin is then eluted and recovered. (AEC)

  11. Fissioning in planarians: control by the brain.

    PubMed

    Best, J B; Goodman, A B; Pigon, A

    1969-05-01

    Reduced population densities lead to increased rates of fissioning in planarians whereas higher population densities suppress fissioning. This effect is not primarily due to mucus deposition or substances secreted into the water. Experiments are presented which show a system of population feedback control. In the presence of other planarians, the brain exerts an influence (probably neurohormonal) to suppress fissioning. This influence becomes attenuated with axial distance from the brain.

  12. Fission-product retention in HTGR fuels

    SciTech Connect

    Homan, F.J.; Kania, M.J.; Tiegs, T.N.

    1982-01-01

    Retention data for gaseous and metallic fission products are presented for both Triso-coated and Biso-coated HTGR fuel particles. Performance trends are established that relate fission product retention to operating parameters, such as temperature, burnup, and neutron exposure. It is concluded that Biso-coated particles are not adequately retentive of fission gas or metallic cesium, and Triso-coated particles which retain cesium still lose silver. Design implications related to these performance trends are identified and discussed.

  13. Fission Product Decay Heat Calculations for Neutron Fission of 232Th

    NASA Astrophysics Data System (ADS)

    Son, P. N.; Hai, N. X.

    2016-06-01

    Precise information on the decay heat from fission products following times after a fission reaction is necessary for safety designs and operations of nuclear-power reactors, fuel storage, transport flasks, and for spent fuel management and processing. In this study, the timing distributions of fission products' concentrations and their integrated decay heat as function of time following a fast neutron fission reaction of 232Th were exactly calculated by the numerical method with using the DHP code.

  14. FISSION PRODUCT REMOVAL FROM ORGANIC SOLUTIONS

    DOEpatents

    Moore, R.H.

    1960-05-10

    The decontamination of organic solvents from fission products and in particular the treatment of solvents that were used for the extraction of uranium and/or plutonium from aqueous acid solutions of neutron-irradiated uranium are treated. The process broadly comprises heating manganese carbonate in air to a temperature of between 300 and 500 deg C whereby manganese dioxide is formed; mixing the manganese dioxide with the fission product-containing organic solvent to be treated whereby the fission products are precipitated on the manganese dioxide; and separating the fission product-containing manganese dioxide from the solvent.

  15. First results from the new double velocity-double energy spectrometer VERDI

    NASA Astrophysics Data System (ADS)

    Frégeau, M. O.; Oberstedt, S.; Gamboni, Th.; Geerts, W.; Hambsch, F.-J.; Vidali, M.

    2016-05-01

    The VERDI spectrometer (VElocity foR Direct mass Identification) is a two arm time-of-flight spectrometer built at the European Commission Joint Research Centre IRMM. It determines fragment masses and kinetic energy distributions produced in nuclear fission by means of the double velocity and double energy (2v-2E) method. The simultaneous measurement of pre- and post neutron fragment characteristics allows studying the share of excitation energy between the two fragments. In particular, the evolution of fission modes and neutron multiplicity may be studied as a function of the available excitation energy. Both topics are of great importance for the development of models used in the evaluation of nuclear data, and also have important implications for the fundamental understanding of the fission process. The development of VERDI focus on maximum geometrical efficiency while striving for highest possible mass resolution. An innovative transmission start detector, using electrons ejected from the target itself, was developed. Stop signal and kinetic energy of both fragments are provided by two arrays of silicon detectors. The present design provides about 200 times higher geometrical efficiency than that of the famous COSI FAN TUTTE spectrometer [Nuclear Instruments and Methods in Physics Research 219 (1984) 569]. We report about a commissioning experiment of the VERDI spectrometer, present first results from a 2v-2E measurement of 252Cf spontaneous fission and discuss the potential of this instrument to contribute to the investigation prompt fission neutron characteristics as a function of fission fragment properties.

  16. A hemi-fission intermediate links two mechanistically distinct stages of membrane fission

    PubMed Central

    Sundborger, Anna C.; Hortelano, Eva Rodriguez; Fuhrmans, Marc; Neumann, Sylvia; Müller, Marcus; Hinshaw, Jenny E.; Schmid, Sandra L.; Frolov, Vadim A.

    2015-01-01

    Fusion and fission drive all vesicular transport. Although topologically opposite, these reactions pass through the same hemi-fusion/fission intermediate1,2, characterized by a ‘stalk’ in which only the inner monolayers of the two compartments have merged to form a localized non-bilayer connection1-3. Formation of the hemi-fission intermediate requires energy input from proteins catalyzing membrane remodeling; however the relationship between protein conformational rearrangements and hemi-fusion/fission remains obscure. Here we analyzed how the GTPase cycle of dynamin, the prototypical membrane fission catalyst4-6, is directly coupled to membrane remodeling. We used intra-molecular chemical cross-linking to stabilize dynamin in its GDP•AlF4--bound transition-state. In the absence of GTP this conformer produced stable hemi-fission, but failed to progress to complete fission, even in the presence of GTP. Further analysis revealed that the pleckstrin homology domain (PHD) locked in its membrane-inserted state facilitated hemi-fission. A second mode of dynamin activity, fueled by GTP hydrolysis, couples dynamin disassembly with cooperative diminishing of the PHD wedging, thus destabilizing the hemi-fission intermediate to complete fission. Molecular simulations corroborate the bimodal character of dynamin action and indicate radial and axial forces as dominant, although not independent drivers of hemi-fission and fission transformations, respectively. Mirrored in the fusion reaction7-8, the force bimodality might constitute a general paradigm for leakage-free membrane remodeling. PMID:26123023

  17. METHOD FOR SEPARATING PLUTONIUM AND FISSION PRODUCTS EMPLOYING AN OXIDE AS A CARRIER FOR FISSION PRODUCTS

    DOEpatents

    Davies, T.H.

    1961-07-18

    Carrier precipitation processes for separating plutonium values from uranium fission products are described. Silicon dioxide or titanium dioxide in a finely divided state is added to an acidic aqueous solution containing hexavalent plutonium ions together with ions of uranium fission products. The supernatant solution containing plutonium ions is then separated from the oxide and the fission products associated therewith.

  18. Fission fragment excited laser system

    DOEpatents

    McArthur, David A.; Tollefsrud, Philip B.

    1976-01-01

    A laser system and method for exciting lasing action in a molecular gas lasing medium which includes cooling the lasing medium to a temperature below about 150 K and injecting fission fragments through the lasing medium so as to preferentially excite low lying vibrational levels of the medium and to cause population inversions therein. The cooled gas lasing medium should have a mass areal density of about 5 .times. 10.sup.-.sup.3 grams/square centimeter, relaxation times of greater than 50 microseconds, and a broad range of excitable vibrational levels which are excitable by molecular collisions.

  19. Adsorption and excess fission xenon

    NASA Technical Reports Server (NTRS)

    Podosek, F. A.; Bernatowicz, T. J.; Kramer, F. E.

    1982-01-01

    The adsorption of Xe and Kr on lunar soil 10084 was measured by a method that employs only very low fractions of monolayer coverage. Results are presented as parameters for calculation of the Henry constant for adsorption as a function of temperature. The adsorption potentials are about 3 kcal/mole for Kr and 5 kcal/mole for Xe; heating the sample in vacuum increased the Xe potential to nearly 7 kcal/mole. Henry constants at the characteristic lunar temperature are about 0.3 cu cm STP/g-atm. These data were applied to consider whether adsorption is important in producing the excess fission Xe effect characteristic of highland breccias. Sorption equilibrium with a transient lunar atmosphere vented fission Xe produces concentrations seven orders of magnitude lower than observed concentrations. Higher concentrations result because of the resistance of the regolith to upward diffusion of Xe. A diffusion coefficient of 0.26 sq cm/sec is estimated for this process.

  20. Fission Models of Population Variability

    PubMed Central

    Thompson, E. A.

    1979-01-01

    Most models in population genetics are models of allele frequency, making implicit or explicit assumptions of equilibrium or constant population size. In recent papers, we have attempted to develop more appropriate models for the analysis of rare variant data in South American Indian tribes; these are branching process models for the total number of replicates of a variant allele. The spatial distribution of a variant may convey information about its history and characteristics, and this paper extends previous models to take this factor into consideration. A model of fission into subdivisions is superimposed on the previous branching process, and variation between subdivisions is considered. The case where fission is nonrandom and the locations of like alleles are initially positively associated, as would happen were a tribal cluster or village to split on familial lines, is also analyzed. The statistics developed are applied to Yanomama Indian data on rare genetic variants. Due to insufficient time depth, no definitive new inferences can be drawn, but the analysis shows that this model provides results consistent with previous conclusions, and demonstrates the general type of question that may be answered by the approach taken here. In particular, striking confirmation of a higher-than-average growth rate, and hence smaller-than-previously-estimated age, is obtained for the Yan2 serum albumen variant. PMID:535728

  1. Spontaneous periodic hypothermia.

    PubMed

    Kloos, R T

    1995-09-01

    Spontaneous periodic hypothermia is a rare syndrome of recurrent, centrally mediated hypothermia without an identifiable systemic cause or brain lesion. Most patients defend a temporarily lowered temperature "set point" during episodes of hypothermia, despite manifesting many well-known systemic consequences of core temperature hypothermia. No case of death directly attributable to an episode of spontaneous periodic hypothermia has been reported, although many of the serious systemic effects of hypothermia have been documented in these cases, so it is not unlikely that death may occur. The syndrome's cause, and that of Shapiro syndrome, remains unknown. Pharmacologic trials to date have been only modestly successful. Anticonvulsant agents, clonidine, and cyproheptadine appear the most likely to succeed, with cyproheptadine being a reasonable first choice. Given that the term "spontaneous periodic hypothermia" describes a syndrome, and not a pathophysiologic mechanism, it is likely to encompass a common eventuality, arrived at via several different pathways. One can postulate mechanisms such as structural abnormalities, trauma, infection, irritation, and degeneration involving strategic locations which create a focus for epileptic or other periodic dysfunction whose scope involves the centers for thermoregulation. The existence of 2 distinct, oppositional thermoregulatory centers would allow for speculation of similar mechanisms accounting for cases of both periodic hypo- and hyperthermia (61). Postmortem data regarding the hypothalamic and surrounding areas from future cases of Shapiro syndrome and spontaneous periodic hypothermia would be of great interest. Further, more sensitive in vivo testing methods are clearly needed. The role of PET or single photon emission computed tomography (SPECT) with technetium 99m-labeled hexamethylpropylene amine oxime (Tc 99m HMPAO) performed acutely during an episode remains to be characterized (64, 103, 105). The term

  2. Spectrum of carbonaceous-chondrite fission xenon

    NASA Technical Reports Server (NTRS)

    Clayton, D. D.

    1976-01-01

    Estimations of the fission spectrum in xenon isotopes from the progenitor of the strange carbonaceous-chondrite xenon must take account of p-process nucleosynthesis if the latter is the source of anomalous Xe-124, 126. Sample calculations of the p-process yields illustrate the magnitude of the effect, which can greatly increase the estimated Xe-132 fission yield.

  3. Options for Affordable Fission Surface Power Systems

    NASA Technical Reports Server (NTRS)

    Houts, Mike; Gaddis, Steve; Porter, Ron; VanDyke, Melissa; Martin Jim; Godfroy, Tom; Bragg-Sitton, Shannon; Garber, Anne; Pearson, Boise

    2006-01-01

    Fission surface power systems could provide abundant power anywhere on free surface of the moon or Mars. Locations could include permanently shaded regions on the moon and high latitudes on Mars. To be fully utilized; however, fission surface power systems must be safe, have adequate performance, and be affordable. This paper discusses options for the design and development of such systems.

  4. PROCESS FOR SEPARATING URANIUM FISSION PRODUCTS

    DOEpatents

    Spedding, F.H.; Butler, T.A.; Johns, I.B.

    1959-03-10

    The removal of fission products such as strontium, barium, cesium, rubidium, or iodine from neutronirradiated uranium is described. Uranium halide or elemental halogen is added to melted irradiated uranium to convert the fission products to either more volatile compositions which vaporize from the melt or to higher melting point compositions which separate as solids.

  5. Prompt fission neutron spectra of actinides

    DOE PAGES

    Capote, R.; Chen, Y. -J.; Hambsch, F. -J.; Kornilov, N. V.; Lestone, J. P.; Litaize, O.; Morillon, B.; Neudecker, D.; Oberstedt, S.; Ohsawa, T.; et al

    2016-01-06

    Here, the energy spectrum of prompt neutrons emitted in fission (PFNS) plays a very important role in nuclear science and technology. A Coordinated Research Project (CRP) "Evaluation of Prompt Fission Neutron Spectra of Actinides" was established by the IAEA Nuclear Data Section in 2009, with the major goal to produce new PFNS evaluations with uncertainties for actinide nuclei.

  6. Nuclear Power from Fission Reactors. An Introduction.

    ERIC Educational Resources Information Center

    Department of Energy, Washington, DC. Technical Information Center.

    The purpose of this booklet is to provide a basic understanding of nuclear fission energy and different fission reaction concepts. Topics discussed are: energy use and production, current uses of fuels, oil and gas consumption, alternative energy sources, fossil fuel plants, nuclear plants, boiling water and pressurized water reactors, the light…

  7. Options for Affordable Fission Surface Power Systems

    SciTech Connect

    Houts, Mike; Gaddis, Steve; Porter, Ron; Van Dyke, Melissa; Martin, Jim; Godfroy, Tom; Bragg-Sitton, Shannon; Garber, Anne; Pearson, Boise

    2006-07-01

    Fission surface power systems could provide abundant power anywhere on the surface of the moon or Mars. Locations could include permanently shaded regions on the moon and high latitudes on Mars. To be fully utilized, however, fission surface power systems must be safe, have adequate performance, and be affordable. This paper discusses options for the design and development of such systems. (authors)

  8. SOURCE OF PRODUCTS OF NUCLEAR FISSION

    DOEpatents

    Harteck, P.; Dondes, S.

    1960-03-15

    A source of fission product recoil energy suitable for use in radiation chemistry is reported. The source consists of thermal neutron irradiated glass wool having a diameter of 1 to 5 microns and containing an isotope fissionable by thermal neutrons, such as U/sup 235/.

  9. Fission Surface Power Technology Development Status

    NASA Technical Reports Server (NTRS)

    Palac, Donald T.; Mason, Lee S.; Houts, Michael G.; Harlow, Scott

    2010-01-01

    Power is a critical consideration in planning exploration of the surfaces of the Moon, Mars, and beyond. Nuclear power is an important option, especially for locations in the solar system where sunlight is limited in availability or intensity. NASA is maintaining the option for fission surface power for the Moon and Mars by developing and demonstrating technology for an affordable fission surface power system. Because affordability drove the determination of the system concept that this technology will make possible, low development and recurring costs result, while required safety standards are maintained. However, an affordable approach to fission surface power also provides the benefits of simplicity, robustness, and conservatism in design. This paper will illuminate the multiplicity of benefits to an affordable approach to fission surface power, and will describe how the foundation for these benefits is being developed and demonstrated in the Exploration Technology Development Program s Fission Surface Power Project.

  10. Fission dynamics at low excitation energy

    NASA Astrophysics Data System (ADS)

    Aritomo, Y.; Chiba, S.; Ivanyuk, F.

    2014-11-01

    The mass asymmetry in the fission of 236U at low excitation energy is clarified by the analysis of the trajectories obtained by solving the Langevin equations for the shape degrees of freedom. It is demonstrated that the position of the peaks in the mass distribution of fission fragments is determined mainly by the saddle point configuration originating from the shell correction energy. The width of the peaks, on the other hand, results from the shape fluctuations close to the scission point caused by the random force in the Langevin equation. We have found out that the fluctuations between elongated and compact shapes are essential for the fission process. According to our results the fission does not occur with continuous stretching in the prolate direction, similarly to that observed in starch syrup, but is accompanied by the fluctuations between elongated and compact shapes. This picture presents a new viewpoint of fission dynamics and the splitting mechanism.

  11. Investigations of fission characteristics and correlation effects

    NASA Astrophysics Data System (ADS)

    Gundorin, N. A.; Zeinalov, Sh. S.; Kopach, Yu. N.; Popov, A. B.; Furman, V. I.

    2016-07-01

    We review the experimental results on the P-even and P-odd angular correlations of fission fragments in the fission of the 235U and 239Pu nuclei induced by unpolarized and polarized resonance neutrons, and on the TRI and ROT effects in the ternary and binary fission of actinides induced by polarized thermal neutrons. Also reported are the measured yields of prompt and delayed neutrons per fission event. The experimental data are analyzed within a novel theoretical framework developed by the JINR—RNC KI Collaboration, whereby the reduction of the multidimensional phase space of fission fragments to the JπK-channel space is consistently validated and the role of resonance interference in the observed correlation effects is revealed.

  12. Spontaneous ileostomy closure

    PubMed Central

    Alyami, Mohammad S.; Lundberg, Peter W.; Cotte, Eddy G.; Glehen, Olivier J.

    2016-01-01

    Iatrogenic ileostomies are routinely placed during colorectal surgery for the diversion of intestinal contents to permit healing of the distal anastomosis prior to elective reversal. We present an interesting case of spontaneous closure of a diverting ileostomy without any adverse effects to the patient. A 65-year-old woman, positive for hereditary non-polyposis colorectal cancer type-I, with locally invasive cancer of the distal colon underwent en-bloc total colectomy, hysterectomy, and bilateral salpingoophorectomy with creation of a proximal loop ileostomy. The ostomy temporarily closed without reoperation at 10 weeks, after spontaneously reopening, it definitively closed, again without surgical intervention at 18 weeks following the original surgery. This rare phenomenon has occurred following variable colorectal pathology and is poorly understood, particularly in patients with aggressive disease and adjunct perioperative interventions. PMID:27279518

  13. Spontaneous Transomental Hernia

    PubMed Central

    Lee, Seung Hun

    2016-01-01

    A transomental hernia through the greater or lesser omentum is rare, accounting for approximately 4% of internal hernias. Transomental hernias are generally reported in patients aged over fifty. In such instances, acquired transomental hernias are usual, are commonly iatrogenic, and result from surgical interventions or from trauma or peritoneal inflammation. In rare cases, such as the one described in this study, internal hernias through the greater or lesser omentum occur spontaneously as the result of senile atrophy without history of surgery, trauma, or inflammation. A transomental hernia has a high postoperative mortality rate of 30%, and emergency diagnosis and treatment are critical. We report a case of a spontaneous transomental hernia of the small intestine causing intestinal obstruction. An internal hernia with strangulation of the small bowel in the lesser sac was suspected from the image study. After an emergency laparotomy, a transomental hernia was diagnosed. PMID:26962535

  14. [Spontaneous bilateral Petit hernia].

    PubMed

    Fontoura, Rodrigo Dias; Araújo, Emerson Silveira de; Oliveira, Gustavo Alves de; Sarmenghi Filho, Deolindo; Kalil, Mitre

    2011-01-01

    Petit's lumbar hernia is an uncommon defect of the posterior abdominal wall that represents less than 1% of all abdominal wall hernias. It is more often unilateral and founded in young females, rarely containing a real herniated sac. There are two different approaches to repair: laparoscopy and open surgery. The goal of this article is to report one case of spontaneous bilateral lumbar Petit's hernia treated with open surgery.

  15. Overview of fission yeast septation.

    PubMed

    Pérez, Pilar; Cortés, Juan C G; Martín-García, Rebeca; Ribas, Juan C

    2016-09-01

    Cytokinesis is the final process of the vegetative cycle, which divides a cell into two independent daughter cells once mitosis is completed. In fungi, as in animal cells, cytokinesis requires the formation of a cleavage furrow originated by constriction of an actomyosin ring which is connected to the plasma membrane and causes its invagination. Additionally, because fungal cells have a polysaccharide cell wall outside the plasma membrane, cytokinesis requires the formation of a septum coincident with the membrane ingression. Fission yeast Schizosaccharomyces pombe is a unicellular, rod-shaped fungus that has become a popular model organism for the study of actomyosin ring formation and constriction during cell division. Here we review the current knowledge of the septation and separation processes in this fungus, as well as recent advances in understanding the functional interaction between the transmembrane enzymes that build the septum and the actomyosin ring proteins. PMID:27155541

  16. Fission-track dating of apatite and zircon: An interlaboratory comparison

    USGS Publications Warehouse

    Naeser, C.W.; Zimmermann, R.A.; Cebula, G.T.

    1981-01-01

    Apatite and zircon separates from the Fish Canyon Tuff (K-Ar age, 27.9??0.7 Myr), San Juan Mtns., Colorado, have been given to over 50 laboratories for fission-track dating. Nineteen laboratories have reported fission-track ages that they have determined for apatites. Nine laboratories have reported their analysis of the zircons. The principal difference between the results reported by the laboratories reflects their choice of the decay constant. The laboratories which use a value of ??f ??? 7.0 ?? 10-17 yr-1 for the spontaneous-fission decay constant of 238U, report an average age for the apatite of 28.5??0.7 Myr, and those using ??f ??? = 8.4 ?? 10-17 yr-1 report an average age of 23.6??1.0 Myr. The average fission-track age for the zircons is 28.4??0.7 Myr. Only laboratories which use ??f ??? 7.0 ?? 10-17 yr-1 reported zircon data. ?? 1981.

  17. Dating thermal events at Cerro Prieto using fission-track annealing

    SciTech Connect

    Sanford, S.J.; Elders, W.A.

    1981-01-01

    The duration of heating in the Cerro Prieto reservoir was estimated by relating the fading of spontaneous fission tracks in detrital apatite to observed temperatures. The rate of fading is a function of both time and temperature. The apparent fission track age of the detrital apatites then, is a function of both their source age and their time-temperature history. Data from laboratory experiments and geologic fading studies were compiled from published sources to produce lines of iso-annealing for apatite in time-temperature space. Fission track ages were calculated for samples from two wells at Cerro Prieto, one with an apparently simple and one with an apparently complex thermal history. Temperatures were estimated by empirical vitrinite reflectance geothermometry, fluid inclusion homogenization and oxygen isotope equilibrium. These estimates were compared with logs of measured borehole temperatures. The temperature in well T-366, where complete annealing first occurs, was estimated to be between 160 and 180{sup 0}C. Complete annealing at these temperatures requires 10{sup 4} and 10{sup 3} years, respectively. Well M-94 has an apparently complex thermal history. Geothermometers in this well indicate temperatures some 50 to 100{sup 0}C higher than those measured directly in the borehole. Fission tracks are partially preserved in M-94 where paleotemperatures were as high as 200{sup 0}C and are erased where geothermometers indicate temperatures of 250{sup 0}C. This implies a thermal event less than 10{sup 1} years and greater than 10{sup 0} years in duration.

  18. Fifty years with nuclear fission. Volume 2

    SciTech Connect

    Behrens, J.W.; Carlson, A.D.

    1989-12-31

    The news of the discovery of nucler fission, by Otto Hahn and Fritz Strassmann in Germany, was brought to the United States by Niels Bohr in January 1939. Since its discovery, the United States, and the world for that matter, has never been the same. It therefore seemed appropriate to acknowledge the fiftieth anniversary of its discovery by holding a topical meeting entitled, ``Fifty years with nuclear fission,`` in the United States during the year 1989. The objective of the meeting was to bring together pioneers of the nuclear industry and other scientists and engineers to report on reminiscences of the past and on the more recent developments in fission science and technology. The conference highlighted the early pioneers of the nuclear industry by dedicating a full day (April 26), consisting of two plenary sessions, at the National Academy of Sciences (NAS) in Washington, DC. More recent developments in fission science and technology in addition to historical reflections were topics for two full days of sessions (April 27 and 28) at the main sites of the NIST in Gaithersburg, Maryland. The wide range of topics covered by Volume 2 of this topical meeting included plenary invited, and contributed sessions entitled, Nuclear fission -- a prospective; reactors II; fission science II; medical and industrial applications by by-products; reactors and safeguards; general research, instrumentation, and by-products; and fission data, astrophysics, and space applications. The individual papers have been cataloged separately.

  19. Gas-phase chemistry of technetium carbonyl complexes.

    PubMed

    Wang, Yang; Qin, Zhi; Fan, Fang-Li; Haba, Hiromitsu; Komori, Yukiko; Cao, Shi-Wei; Wu, Xiao-Lei; Tan, Cun-Min

    2015-05-28

    Gas-phase chemical behaviors of short-lived technetium carbonyl complexes were studied using a low temperature isothermal chromatograph (IC) coupled with a (252)Cf spontaneous fission (SF) source. Fission products recoiled from the (252)Cf SF source were thermalized in a mixed gas containing CO, and then technetium carbonyl complexes were formed from reactions between CO gas and various technetium isotopes. A gas-jet system was employed to transport the volatile carbonyl complexes from a recoil chamber to the IC. Short IC columns made of Fluorinated Ethylene Propylene (FEP) Teflon and quartz were used to obtain chemical information about the technetium carbonyl complexes. The results for the (104)Tc-(106)Tc carbonyl complexes were found to be strongly influenced by the precursors, and showed the chemical behaviors of (104)Mo-(106)Mo carbonyl complexes, respectively. However, (107)Tc and (108)Tc could represent the chemical information of the element technetium due to their high independent yields and the very short half-lives of their precursors (107)Mo and (108)Mo. An adsorption enthalpy of about ΔHads = -43 kJ mol(-1) was determined for the Tc carbonyl complexes on both the Teflon and quartz surfaces by fitting the breakthrough curves of the (107)Tc and (108)Tc carbonyl complexes with a Monte Carlo simulation program. Chemical yields of around 25% were measured for the Tc carbonyl complexes relative to the transport yields obtained with the gas-jet transport of KCl aerosol particles with Ar carrier gas. Furthermore, the influence of a small amount of O2 gas on the yields of the Mo and Tc carbonyl complexes was studied.

  20. Active neutron interrogation for verification of storage of weapons components at the Oak Ridge Y-12 Plant

    SciTech Connect

    Mihalczo, J.T.; Valentine, T.E.; Mattingly, J.K.; Mullens, J.A.; Hughes, S.S.

    1998-02-23

    A nuclear weapons identification system (NWIS), under development since 1984 at the Oak Ridge Y-12 Plant and presently in use there, uses active neutron interrogation with low-intensity {sup 252}Cf sources in ionization chambers to provide a timed source of fission neutrons from the spontaneous fission of {sup 252}Cf. To date, measurements have been performed on {approximately}15 different weapons systems in a variety of configurations both in and out of containers. Those systems included pits and fully assembled systems ready for deployment at the Pantex Plant in Amarillo, Texas, and weapons components at the Oak Ridge Y-12 Plant. These measurements have shown that NWIS can identify nuclear weapons and/or components; nuclear weapons/components can be distinguished from mockups where fissile material has been replaced by nonfissile material; omissions of small amounts (4%) of fissile material can be detected; changes in internal configurations can be determined; trainer parts can be identified as was demonstrated by verification of 512 containers with B33 components at the Y-12 Plant (as many as 32 in one 8-hour shift); and nonfissile components can be identified. The current NWIS activities at the Oak Ridge Y-12 Plant include: (1) further development of the system for more portability and lower power consumption, (2) collection of reference signatures for all weapons components in containers, and (3) confirmation of a particular weapons component in storage and confirmation of receipts. This paper describes the recent measurements with NWIS for a particular weapons component in storage that have resolved an Inspector General (IG`s) audit finding with regard to performance of confirmation of inventory.

  1. Gas-phase chemistry of technetium carbonyl complexes.

    PubMed

    Wang, Yang; Qin, Zhi; Fan, Fang-Li; Haba, Hiromitsu; Komori, Yukiko; Cao, Shi-Wei; Wu, Xiao-Lei; Tan, Cun-Min

    2015-05-28

    Gas-phase chemical behaviors of short-lived technetium carbonyl complexes were studied using a low temperature isothermal chromatograph (IC) coupled with a (252)Cf spontaneous fission (SF) source. Fission products recoiled from the (252)Cf SF source were thermalized in a mixed gas containing CO, and then technetium carbonyl complexes were formed from reactions between CO gas and various technetium isotopes. A gas-jet system was employed to transport the volatile carbonyl complexes from a recoil chamber to the IC. Short IC columns made of Fluorinated Ethylene Propylene (FEP) Teflon and quartz were used to obtain chemical information about the technetium carbonyl complexes. The results for the (104)Tc-(106)Tc carbonyl complexes were found to be strongly influenced by the precursors, and showed the chemical behaviors of (104)Mo-(106)Mo carbonyl complexes, respectively. However, (107)Tc and (108)Tc could represent the chemical information of the element technetium due to their high independent yields and the very short half-lives of their precursors (107)Mo and (108)Mo. An adsorption enthalpy of about ΔHads = -43 kJ mol(-1) was determined for the Tc carbonyl complexes on both the Teflon and quartz surfaces by fitting the breakthrough curves of the (107)Tc and (108)Tc carbonyl complexes with a Monte Carlo simulation program. Chemical yields of around 25% were measured for the Tc carbonyl complexes relative to the transport yields obtained with the gas-jet transport of KCl aerosol particles with Ar carrier gas. Furthermore, the influence of a small amount of O2 gas on the yields of the Mo and Tc carbonyl complexes was studied. PMID:25920667

  2. Study of the fission isomer 240mAm (S. F. ) using laser-induced nuclear polarization. [Cross section of 238U(7Li,5n) at 48 MeV

    SciTech Connect

    Beene, J. R.; Bemis, Jr., C. E.; Young, J. P.; Kramer, S. D.

    1980-01-01

    The optical isomer shift was measured for the spontaneously fissioning isomer /sup 240m/Am. This shift is approximately 27 times greater than the /sup 241/Am-/sup 243/Am isotope shift, and confirms the conventional identification of fission isomers with large deformation. The measured isomer shift is consistent with a nuclear quadrupole moment of 30.4 b, in agreement with theoretical expectations. 2 figures. (RWR)

  3. Low energy fission: dynamics and scission configurations

    NASA Astrophysics Data System (ADS)

    Goutte, H.; Berger, J.-F.; Gogny, D.; Younes, W.

    2005-11-01

    In the first part of this paper we recall a recent study concerning low energy fission dynamics. Propagation is made by use of the Time Dependent Generator Coordinate Method, where the basis states are taken from self-consistent Hartree-Fock-Bogoliubov calculations with the Gogny force. Theoretical fragment mass distributions are presented and compared with the evaluation made by Wahl. In the second part of this paper, new results concerning scission configurations are shown. Deviations of the fission fragment proton numbers from the Unchanged Charge Distribution prescription and fission fragment deformations are discussed.

  4. Macroscopic and microscopic aspects in nuclear fission

    NASA Astrophysics Data System (ADS)

    Strutinsky, V.

    1989-10-01

    Nuclear macroscopic properties are determined as statistical averages and it is then recognized that several levels of macroscopic descriptions may exist. By zooming the averaging scale the gross shell structures are distinguished from the macroscopic background and a theory can be formed consistently combining both the macroscopic and microscopic features. The shell structure varies in the fissioning nucleus on its way to scission leading to a double-humped shape of the fission barrier. This is due to modifications of the classical periodic paths responsible for the quantal non-uniformity of the single-particle phase space. Briefly results of the combined theory for the fission process are outlined.

  5. [Recurrent spontaneous abortions].

    PubMed

    Salat-Baroux, J

    1988-01-01

    The process of fertilization in humans, is remarkably inefficient. Spontaneous abortion is estimated to be between 15 and 20% of all clinical pregnancies, and the early spontaneous abortion rate is closer to 30-50% of fertilized ova. Not all authors agree on the definition of "recurrent spontaneous abortion" (RSA), so the frequency of repeated pregnancy wastage is difficult to determine; from empirically derived data, it has been estimated to range between 0.4 and 0.8%. Because of the various etiologies of RSA, their association in determining an abortive event, it is difficult to evaluate their exact incidence. Moreover, their is no prospective study on this subject, so it is advisable to distinguish between the admitted causes, the likely factors, and the etiologies to be evaluated. In the first group, the congenital or acquired müllerian anomalies (especially the septate uterus), represent about 25% of the RSA, but a lot of problems concerning the physiopathology are still debated, even if the rate of pregnancies after surgery ranges around 50% in certain series. On the other hand, the genetic factors, identified especially with the banding technique, are undeniable: however, although the rate of chromosomal aberrations in the offspring (Monosomy X, Trisony 16, Triploidy) is very high (50 to 60% of spontaneous abortions in the first trimester of pregnancy), when couples with usual abortions are subjected to karyotypic analysis, genetic anomalies (especially translocations) are been noted in only 6.2% of the women and 2.6% of the men. In the second group, the infective factors (chlamydiae, toxoplasma and mycoplasma) are difficult to analyse since the serology is not sufficient without a real proof of an endometrial colonization. Among the endocrinological causes, the classical luteal phase deficiency remains a subject of controversy (estimated between 3 and 30%) not only for the establishment of the diagnosis, but also for the efficiency of progesterone

  6. Spontaneous acalculous gallbladder perforation

    PubMed Central

    Sheridan, David; Qazi, Almas; Lisa, Selina; Vashisht, Rajiv

    2014-01-01

    An 86-year-old woman, 4 days post-operative following a right-sided Austin-Moore arthroplasty, reported abdominal pain around a known umbilical hernia and became increasingly confused. A diagnosis of incarcerated umbilical hernia was made. At surgery, on entering the peritoneal cavity, bile was immediately noted. The operation was converted to a laparotomy and a perforation was noted in the gallbladder. An open cholecystectomy was performed. Macroscopically the gallbladder was perforated in multiple places, was thin walled and did not contain gallstones. This case demonstrates the difficulty in diagnosing an apparently spontaneous gallbladder perforation in a cognitively frail patient. PMID:25293685

  7. Spontaneous Symmetry Breaking

    NASA Astrophysics Data System (ADS)

    Strocchi, Franco

    One of the most powerful ideas of modern theoretical physics is the mechanism of spontaneous symmetry breaking. It is at the basis of most of the recent achievements in the description of phase transitions in Statistical Mechanics as well as of collective phenomena in solid state physics. It has also made possible the unification of weak, electromagnetic and strong interactions in elementary particle physics. Philosophically, the idea is very deep and subtle (this is probably why its exploitation is a rather recent achievement) and the popular accounts do not fully do justice to it.

  8. Spontaneous acalculous gallbladder perforation.

    PubMed

    Sheridan, David; Qazi, Almas; Lisa, Selina; Vashisht, Rajiv

    2014-10-07

    An 86-year-old woman, 4 days post-operative following a right-sided Austin-Moore arthroplasty, reported abdominal pain around a known umbilical hernia and became increasingly confused. A diagnosis of incarcerated umbilical hernia was made. At surgery, on entering the peritoneal cavity, bile was immediately noted. The operation was converted to a laparotomy and a perforation was noted in the gallbladder. An open cholecystectomy was performed. Macroscopically the gallbladder was perforated in multiple places, was thin walled and did not contain gallstones. This case demonstrates the difficulty in diagnosing an apparently spontaneous gallbladder perforation in a cognitively frail patient.

  9. Future challenges for nuclear data research in fission (u)

    SciTech Connect

    Chadwick, Mark B

    2010-01-01

    I describe some high priority research areas in nuclear fission, where applications in nuclear reactor technologies and in modeling criticality in general are demanding higher accuracies in our databases. We focus on fission cross sections, fission neutron spectra, and fission product data.

  10. A new fission chamber dedicated to Prompt Fission Neutron Spectra measurements

    NASA Astrophysics Data System (ADS)

    Taieb, J.; Laurent, B.; Bélier, G.; Sardet, A.; Varignon, C.

    2016-10-01

    New fission chambers dedicated to Prompt Fission Neutron Spectra measurements with the time-of-flight technique have been developed. The actinide mass embedded in the chamber was maximized, while the alpha-fission discrimination and the time resolution were optimized. Moreover, to reduce the neutron background and spectra distortions, neutron scattering with the materials were minimized by the choice of material and structure. These chambers were then tested and validated during tests and in-beam experiments.

  11. Fission dynamics within time-dependent Hartree-Fock. II. Boost-induced fission

    NASA Astrophysics Data System (ADS)

    Goddard, Philip; Stevenson, Paul; Rios, Arnau

    2016-01-01

    Background: Nuclear fission is a complex large-amplitude collective decay mode in heavy nuclei. Microscopic density functional studies of fission have previously concentrated on adiabatic approaches based on constrained static calculations ignoring dynamical excitations of the fissioning nucleus and the daughter products. Purpose: We explore the ability of dynamic mean-field methods to describe induced fission processes, using quadrupole boosts in the nuclide 240Pu as an example. Methods: Following upon the work presented in Goddard et al. [Phys. Rev. C 92, 054610 (2015)], 10.1103/PhysRevC.92.054610, quadrupole-constrained Hartree-Fock calculations are used to create a potential energy surface. An isomeric state and a state beyond the second barrier peak are excited by means of instantaneous as well as temporally extended gauge boosts with quadrupole shapes. The subsequent deexcitation is studied in a time-dependent Hartree-Fock simulation, with emphasis on fissioned final states. The corresponding fission fragment mass numbers are studied. Results: In general, the energy deposited by the quadrupole boost is quickly absorbed by the nucleus. In instantaneous boosts, this leads to fast shape rearrangements and violent dynamics that can ultimately lead to fission. This is a qualitatively different process than the deformation-induced fission. Boosts induced within a finite time window excite the system in a relatively gentler way and do induce fission but with a smaller energy deposition. Conclusions: The fission products obtained using boost-induced fission in time-dependent Hartree-Fock are more asymmetric than the fragments obtained in deformation-induced fission or the corresponding adiabatic approaches.

  12. [Spontaneous course of depression].

    PubMed

    Azorin, J M

    1995-03-01

    The study of the spontaneous course of depressions nowadays comes up against a number of obstacles. The most important of these is the necessity of using untreated cases, which virtually forces the contemporary researcher to refer to studies performed in the pretherapeutic era, if conclusions are not be drawn only from classical descriptions. Unfortunately, these studies are marked by the absence of strict diagnostic criteria, the heterogeneity of patients included in them, the lack of preciseness of evaluations and the primitive statistical methods used. They are concerned essentially with the duration of depressive phases and the factors which influence it. Among these latter are regularly found age, sex, the number of episodes, the duration of the preceding symptom-free interval, the severity and semiology of the attack, heredity, mode of onset, level of intelligence, the presence or absence of associated pathology and the presence or absence of hospitalisation. Chronicization of depression and the factors concerned with it have also been the object of several studies. A small number of investigations compare the course of the illness in untreated populations. The study of the spontaneous course of depression evidences the necessity of having consensus definitions, and may serve as a basis for a better comprehension of the process of cure and of the real impact of therapies designed to treat depression.

  13. Fission yields of In isotopes in the thermal neutron fission of235U

    NASA Astrophysics Data System (ADS)

    Shmid, M.; Engler, G.

    1983-03-01

    Fission yields of124 132In in the thermal neutron fission of235U were determined for the first time. Charge displacements ΔZ= Z p- Z UCD were calculated for the corresponding mass chains. Both fission yields and charge displacement values were compared with those obtained by systematics by Wahl et al. and Wolfsberg. It was found that the fission yields of the In isotopes obey the gaussian distribution. The displacement function of Wolfsberg seems to give the better representation of the experimental results. Half-lives of124 131In were determined from beta decay curves.

  14. Aqueous cutting fluid for machining fissionable materials

    DOEpatents

    Duerksen, Walter K.; Googin, John M.; Napier, Jr., Bradley

    1984-01-01

    The present invention is directed to a cutting fluid for machining fissionable material. The cutting fluid is formed of glycol, water and boron compound in an adequate concentration for effective neutron attenuation so as to inhibit criticality incidents during machining.

  15. The scission point configuration of fissioning nuclei

    NASA Astrophysics Data System (ADS)

    Ivanyuk, Fedir

    2016-06-01

    We define the optimal shape which fissioning nuclei attain just before the scission and calculate the deformation energy as function of the mass asymmetry at the scission point. The calculated deformation energy is used in quasi-static approximation for the estimation of mass distribution, total kinetic and excitation energy of fission fragments, and the total number of prompt neutrons. The calculated results reproduce rather well the experimental data on the position of the peaks in the mass distribution of fission fragments, the total kinetic and excitation energy of fission fragments. The calculated value of neutron multiplicity is somewhat larger than experimental results. The saw-tooth structure of neutron multiplicity is qualitatively reproduced.

  16. Mechanics of Dynamin-Mediated Membrane Fission

    PubMed Central

    Morlot, Sandrine; Roux, Aurélien

    2013-01-01

    In eukaryotic cells, membrane compartments are split into two by membrane fission. This ensures discontinuity of membrane containers and thus proper compartmentalization. The first proteic machinery implicated in catalyzing membrane fission was dynamin. Dynamin forms helical collars at the neck of endocytic buds. This structural feature suggested that the helix of dynamin could constrict in order to promote fission of the enclosed membrane. However, verifying this hypothesis revealed itself to be a challenge, which inspired many in vitro and in vivo studies. The primary goal of this review is to discuss recent structural and physical data from biophysical studies that have refined our understanding of the dynamin mechanism. In addition to the constriction hypothesis, other models have been proposed to explain how dynamin induces membrane fission. We present experimental data supporting these various models and assess which model is the most probable. PMID:23541160

  17. MCNP6 Fission Multiplicity with FMULT Card

    SciTech Connect

    Wilcox, Trevor; Fensin, Michael Lorne; Hendricks, John S.; James, Michael R.; McKinney, Gregg W.

    2012-06-18

    With the merger of MCNPX and MCNP5 into MCNP6, MCNP6 now provides all the capabilities of both codes allowing the user to access all the fission multiplicity data sets. Detailed in this paper is: (1) the new FMULT card capabilities for accessing these different data sets; (2) benchmark calculations, as compared to experiment, detailing the results of selecting these separate data sets for thermal neutron induced fission on U-235.

  18. Modeling Fission Product Sorption in Graphite Structures

    SciTech Connect

    Szlufarska, Izabela; Morgan, Dane; Allen, Todd

    2013-04-08

    The goal of this project is to determine changes in adsorption and desorption of fission products to/from nuclear-grade graphite in response to a changing chemical environment. First, the project team will employ principle calculations and thermodynamic analysis to predict stability of fission products on graphite in the presence of structural defects commonly observed in very high- temperature reactor (VHTR) graphites. Desorption rates will be determined as a function of partial pressure of oxygen and iodine, relative humidity, and temperature. They will then carry out experimental characterization to determine the statistical distribution of structural features. This structural information will yield distributions of binding sites to be used as an input for a sorption model. Sorption isotherms calculated under this project will contribute to understanding of the physical bases of the source terms that are used in higher-level codes that model fission product transport and retention in graphite. The project will include the following tasks: Perform structural characterization of the VHTR graphite to determine crystallographic phases, defect structures and their distribution, volume fraction of coke, and amount of sp2 versus sp3 bonding. This information will be used as guidance for ab initio modeling and as input for sorptivity models; Perform ab initio calculations of binding energies to determine stability of fission products on the different sorption sites present in nuclear graphite microstructures. The project will use density functional theory (DFT) methods to calculate binding energies in vacuum and in oxidizing environments. The team will also calculate stability of iodine complexes with fission products on graphite sorption sites; Model graphite sorption isotherms to quantify concentration of fission products in graphite. The binding energies will be combined with a Langmuir isotherm statistical model to predict the sorbed concentration of fission

  19. A New Simplified System for the Evaluation of BNCT Pharmaceuticals

    SciTech Connect

    Byrne, T.E.; Kabalka, G.W.; Martin, R.C.; Miller, L.F.

    1998-09-13

    A system for testing potential BNCT pharmaceuticals in cell cultures has been developed with the cooperation of Oak Ridge National Laboratory (ORNL), the University of Tennessee Chemistry Department and the University of Tennessee Nuclear Engineering Department. A BNCT test model has been established with the use of the human lung cancer cell line A 549. These cells were maintained in standard laboratory facilities and subjected to boronated chemicals. Following toxicity studies the human luug cancer cells were exposed to {sup 252}Cf neutron sources provided by the Radiochemical Engineering Development Center (REDC) at ORNL The isotope {sup 252}Cf performs effectively for BNCT applications. The neutron spectrum is similar to that of a reactor fission source with an average energy of 2.1 MeV. A 50 mg source of {sup 252}Cf moderated by water provides a source on the order of 1 x 10{sup 9} thermal neutrons/cm{sup 2}/sec at a distance of 3 cm. The half-life of {sup 252}Cf is 2.65 years, and thus may provide a simple and reliable source of neutrons for BNCT in locations without suitable nuclear reactors. The REDC of ORNL stores and processes the U.S. stockpile of {sup 252}Cf.

  20. Ionization Chamber for Prompt Fission Neutron Investigations

    NASA Astrophysics Data System (ADS)

    Zeynalov, Sh.; Zeynalova, O.; Hambsch, F.-J.; Sedyshev, P.; Shvetsov, V.

    In this work we report recent achievements in design of twin back-to-back ionization chamber (TIC) for fission fragment (FF) mass and kinetic energy measurement. Correlated FF kinetic energies, their masses and the angle of FF in respect to the axes in 3D Cartesian coordinates can be determined from analysis of the heights and shapes of the pulses induced by the fission fragments on the anodes of TIC. Anodes of TIC were designed as consisting of isolated strips each having independent electronic circuitry and special multi-channel pulse processing apparatus. Mathematical formulae provided for FF angles measured in respect to the coordinate axes. It was shown how the point of fission fragments origin on the target plane may be determined using the same measured data. The last feature made the TIC a rather powerful tool for prompt fission neutron (PFN) emission investigation in event-by-event analysis of individual fission reactions from non- point fissile source. Position sensitive neutron induced fission detector for neutron-imaging applications with both thermal and low energy neutrons was found as another possible implementation of the designed TIC.

  1. Novel roles for actin in mitochondrial fission

    PubMed Central

    Hatch, Anna L.; Gurel, Pinar S.; Higgs, Henry N.

    2014-01-01

    ABSTRACT Mitochondrial dynamics, including fusion, fission and translocation, are crucial to cellular homeostasis, with roles in cellular polarity, stress response and apoptosis. Mitochondrial fission has received particular attention, owing to links with several neurodegenerative diseases. A central player in fission is the cytoplasmic dynamin-related GTPase Drp1, which oligomerizes at the fission site and hydrolyzes GTP to drive membrane ingression. Drp1 recruitment to the outer mitochondrial membrane (OMM) is a key regulatory event, which appears to require a pre-constriction step in which the endoplasmic reticulum (ER) and mitochondrion interact extensively, a process termed ERMD (ER-associated mitochondrial division). It is unclear how ER–mitochondrial contact generates the force required for pre-constriction or why pre-constriction leads to Drp1 recruitment. Recent results, however, show that ERMD might be an actin-based process in mammals that requires the ER-associated formin INF2 upstream of Drp1, and that myosin II and other actin-binding proteins might be involved. In this Commentary, we present a mechanistic model for mitochondrial fission in which actin and myosin contribute in two ways; firstly, by supplying the force for pre-constriction and secondly, by serving as a coincidence detector for Drp1 binding. In addition, we discuss the possibility that multiple fission mechanisms exist in mammals. PMID:25217628

  2. The Munich Accelerator for Fission Fragments MAFF

    SciTech Connect

    Habs, D.; Gross, M.; Assmann, W.; Beck, L.; Grossmann, R.; Maier, H.-J.; Schumann, M.; Sewtz, M.; Szerypo, J.; Thirolf, P.G.; Kruecken, R.; Faestermann, T.; Maier-Komor, P.; Nebel, F.; Zech, E.; Hartung, P.; Stoepler, R.; Juettner, Ph.; Tralmer, F.L.

    2005-11-21

    The layout and status of MAFF at the Munich high flux reactor FRM-II is described. At MAFF 1014 fissions/s will be induced by thermal neutrons in a target with approx. 1 g of 235U. The situation is compared to the SPIRAL2 facility where 1014 fissions/s are expected by fast neutron fission in a target containing 5100 g of 238U. A comparison of the yields of SPIRAL2 and MAFF is performed to show the complementarity of the two ISOL-facilities for fission fragments. MAFF has approximately five times the beam intensities of SPIRAL2 for short-lived fission isotopes with lifetimes shorter than 5 s and thus will focus on the most neutron-rich nuclei, while SPIRAL2 has better perspectives for the more intense, less neutron-rich post-accelerated beams.A problem that also deserves attention is the production of {alpha} emitters, in particular plutonium. Here MAFF has the advantage to contain the Pu-producing 238U only as impurity not as the main fissile system. If SPIRAL2 would use 235U instead of 238U this problematic issue could be avoided at the cost of a further reduction in intensity of very neutron-rich fission fragments by a factor of 10. Finally new physics close to the classically doubly-magic nuclei 78Ni and 132Sn is described.

  3. Shape Isomers - a Key to Fission Barriers

    NASA Astrophysics Data System (ADS)

    Oberstedt, S.; Hambsch, F.-J.; Kornilov, N.; Lövestam, G.; Oberstedt, A.; Gawrys, M.

    2008-04-01

    Quantitative predictions of fission product yields are relevant for the reliable operation of different modern nuclear applications. This concerns the realistic characterizations of the radio-toxicity of the fuel elements after the envisaged extended irradiation, as well as sub-critical assemblies, where the number of delayed neutrons from minor actinides is determined by the characteristic emission yields of the corresponding so-called pre-cursor isotopes. However, to be able to make more reliable quantitative predictions of fission characteristics requires the better understanding of the fission process itself. For this purpose a better knowledge about the distinct structure of the nuclear energy landscape around the fission barrier is indispensable. In particular, the question should be answered, whether the fission barrier is either double- or triple-humped or even multi-humped as been proposed within the multi-modal neck rupture model. Despite quite some effort based on different experimental techniques and theoretical approaches, this question remains still unanswered. There is still no consistent picture of the fission barrier available and hence, different sets of barrier parameters are in use, unable to describe the different observed phenomena in a coherent way. With the systematic investigation of shape isomer population, its decay modes as well as the branching ratio, precise information can be obtained to resolve the puzzling situation. The experimental approach will be discussed and results from first experiments presented.

  4. Fission-fusion neutron source

    NASA Astrophysics Data System (ADS)

    Yu, Jinnan; Yu, Gang

    2009-04-01

    In order to meet the requirements of fusion power reactors and nuclear waste treatment, a concept of fission-fusion neutron source is proposed, which consists of a LiD assembly located in the heavy water region of the China Advanced Research Reactor. This assembly of LiD fuel rods will be irradiated with slow neutrons and will produce fusion neutrons in the central hole via the reaction 6Li(n, α). More precisely, tritium ions with a high energy of 2.739 MeV will be produced in LiD by the impinging slow neutrons. The tritium ions will in turn bombard the deuterium ions present in the LiD assembly, which will induce fusion reaction and then the production of 14 MeV neutrons. The fusion reaction rate will increase with the accumulation of tritium in LiD by the reaction between tritium and deuteron recoils produced by the 14 MeV neutrons. When the concentration of tritium reaches 0.5 · 10 22 and the fraction of fusion reactions between tritium and deuteron recoils approaches 1, the 14 MeV neutron flux is doubled and redoubled, an so forth, approaching saturation in which the tritium produced at a time t is exhausted by the fusion reactions to keep constant the tritium concentration in LiD.

  5. Further Investigations of NIST Water Sphere Discrepancies

    SciTech Connect

    Broadhead, B.L.

    2001-01-11

    Measurements have been performed on a family of water spheres at the National Institute of Standards and Technology (NIST) facilities. These measurements are important for criticality safety studies in that, frequently, difficulties have arisen in predicting the reactivity of individually subcritical components assembled in a critical array. It has been postulated that errors in the neutron leakage from individual elements in the array could be responsible for these problems. In these NIST measurements, an accurate determination of the leakage from a fission spectrum, modified by water scattering, is available. Previously, results for 3-, 4-, and 5-in. diam. water-filled spheres, both with and without cadmium covers over the fission chambers, were presented for four fissionable materials: {sup 235}U, {sup 238}U, {sup 237}Np, and {sup 239}Pu. Results were also given for ''dry'' systems, in which the water spheres were drained of water, with the results corresponding to essentially measurements of unmoderated {sup 252}Cf spontaneous-fission neutrons. The calculated-to-experimental (C/E) values ranged from 0.94 to 1.01 for the dry systems and 0.93 to 1.05 for the wet systems, with experimental uncertainties ranging from 1.5 to 1.9%. These results indicated discrepancies that were clearly outside of the experimental uncertainties, and further investigation was suggested. This work updates the previous calculations with a comparison of the predicted C/E values with ENDF/B-V and ENDF/B-VI transport cross sections. Variations in the predicted C/E values that arise from the use of ENDF/B-V, ENDF/B-VI, ENDL92, and LLLDOS for the response fission cross sections are also tabulated. The use of both a 45-group NIST fission spectrum and a continuous-energy fission spectrum for {sup 252}Cf are evaluated. The use of the generalized-linear-least-squares (GLLSM) procedures to investigate the reported discrepancies in the water sphere results for {sup 235}U, {sup 238}U, {sup 239}Pu

  6. Spontaneous soft tissue hematomas.

    PubMed

    Dohan, A; Darnige, L; Sapoval, M; Pellerin, O

    2015-01-01

    Spontaneous muscle hematomas are a common and serious complication of anticoagulant treatment. The incidence of this event has increased along with the rise in the number of patients receiving anticoagulants. Radiological management is both diagnostic and interventional. Computed tomography angiography (CTA) is the main tool for the detection of hemorrhage to obtain a positive, topographic diagnosis and determine the severity. Detection of an active leak of contrast material during the arterial or venous phase is an indication for the use of arterial embolization. In addition, the interventional radiological procedure can be planned with CTA. Arterial embolization of the pedicles that are the source of the bleeding is an effective technique. The rate of technical and clinical success is 90% and 86%, respectively. PMID:26066549

  7. Spontaneous Iliac Vein Rupture

    PubMed Central

    Kim, Dae Hwan; Park, Hyung Sub; Lee, Taeseung

    2015-01-01

    Spontaneous iliac vein rupture (SIVR) is a rare entity, which usually occurs without a precipitating factor, but can be a life-threatening emergency often requiring an emergency operation. This is a case report of SIVR in a 62-year-old female who presented to the emergency room with left leg swelling. Workup with contrast-enhanced computed tomography revealed a left leg deep vein thrombosis with May-Thurner syndrome and a hematoma in the pelvic cavity without definite evidence of arterial bleeding. She was managed conservatively without surgical intervention, and also underwent inferior vena cava filter insertion and subsequent anticoagulation therapy for pulmonary thromboembolism. This case shows that SIVR can be successfully managed with close monitoring and conservative management, and anticoagulation may be safely applied despite the patient presenting with venous bleeding. PMID:26217647

  8. Spontaneous Coronary Artery Dissection.

    PubMed

    Tweet, Marysia S; Gulati, Rajiv; Hayes, Sharonne N

    2016-07-01

    Spontaneous coronary artery dissection is an important etiology of nonatherosclerotic acute coronary syndrome, myocardial infarction, and sudden death. Innovations in the catheterization laboratory including optical coherence tomography and intravascular ultrasound have enhanced the ability to visualize intimal disruption and intramural hematoma associated with SCAD. Formerly considered "rare," these technological advances and heightened awareness suggest that SCAD is more prevalent than prior estimates. SCAD is associated with female sex, young age, extreme emotional stress, or extreme exertion, pregnancy, and fibromuscular dysplasia. The clinical characteristics and management strategies of SCAD patients are different than for atherosclerotic heart disease and deserve specific consideration. This review will highlight recent discoveries about SCAD as well as describe current efforts to elucidate remaining gaps in knowledge.

  9. Spontaneous Coronary Artery Dissection.

    PubMed

    Tweet, Marysia S; Gulati, Rajiv; Hayes, Sharonne N

    2016-07-01

    Spontaneous coronary artery dissection is an important etiology of nonatherosclerotic acute coronary syndrome, myocardial infarction, and sudden death. Innovations in the catheterization laboratory including optical coherence tomography and intravascular ultrasound have enhanced the ability to visualize intimal disruption and intramural hematoma associated with SCAD. Formerly considered "rare," these technological advances and heightened awareness suggest that SCAD is more prevalent than prior estimates. SCAD is associated with female sex, young age, extreme emotional stress, or extreme exertion, pregnancy, and fibromuscular dysplasia. The clinical characteristics and management strategies of SCAD patients are different than for atherosclerotic heart disease and deserve specific consideration. This review will highlight recent discoveries about SCAD as well as describe current efforts to elucidate remaining gaps in knowledge. PMID:27216840

  10. Fission-track dating: application to the thermal history of mountains and basins

    SciTech Connect

    Naeser, C.W.; Naeser, N.D.

    1985-01-01

    Fission tracks are cylindrical zones of structural damage found in minerals and glasses. They are formed by the passage of a massive highly-charged ion produced from the spontaneous fission of incorporated /sup 238/U. Fission tracks are stable in most minerals at temperatures <50/sup 0/C, but if a mineral is heated above its track stability zone, the track will fade or anneal. Each mineral species has a characteristic temperature zone over which track annealing takes place, and the extent of this annealing is related to both the temperature and the length of time at that temperature. A short heating event at high temperature will produce the same observed annealing as low temperature heating of long duration. For times greater than approx. =10/sup 6/ years, the temperature range, depending on duration of heating, for total annealing in the three minerals most commonly dated by fission tracks are: apatite 105/sup 0/ to 135/sup 0/C, zircon approx.160/sup 0/ to approx.240/sup 0/C, and sphene approx.250/sup 0/ +/- ./sup 0/C. By looking at the pattern of ages of one or more of these minerals, as a function of depth or elevation, it is possible to determine the paleotemperature history, and the burial or uplift/erosion history, of sedimentary basins and mountain ranges. The distribution of fission-track ages of detrital apatite from Upper Cretaceous and lower Tertiary sedimentary rocks in the Wagon Wheel no. 1 well in the northern Green River basin indicates that these rocks have cooled by at least 20/sup 0/C since the beginning of the Pliocene. Likewise, anomalously young apatite ages from Precambrian rocks at the base of the Wasatch Mountains in Utah show that this range has been uplifted and cooled by at least 100/sup 0/C in the last 5 Ma.

  11. Prompt fission γ -ray spectrum characteristics from 240Pu(sf ) and 242Pu(sf )

    NASA Astrophysics Data System (ADS)

    Oberstedt, S.; Oberstedt, A.; Gatera, A.; Göök, A.; Hambsch, F.-J.; Moens, A.; Sibbens, G.; Vanleeuw, D.; Vidali, M.

    2016-05-01

    In this paper we present first results for prompt fission γ -ray spectra (PFGS) characteristics from the spontaneous fission (sf) of 240Pu and 242Pu. For 242Pu(sf ) we obtained, after proper unfolding of the detector response, an average energy per photon ɛ¯γ=(0.843 ±0.012 ) MeV, an average multiplicity M¯γ=(6.72 ±0.07 ) , and an average total γ -ray energy release per fission E¯γ ,tot = (5.66 ± 0.06) MeV. The 240Pu(sf ) emission spectrum was obtained by applying a so-called detector-response transformation function determined from the 242Pu spectrum measured in exactly the same geometry. The results are an average energy per photon ɛ¯γ=(0.80 ±0.07 ) MeV, the average multiplicity M¯γ = (8.2 ± 0.4), and an average total γ -ray energy release per fission E¯γ ,tot = (6.6 ± 0.5) MeV. The PFGS characteristics for 242Pu(sf ) are in very good agreement with those from thermal-neutron-induced fission on 241Pu and scales well with the corresponding prompt neutron multiplicity. Our results in the case of 240Pu(sf ), although drawn from a limited number of events, show a significantly enhanced average multiplicity and average total energy, but may be understood from a different fragment yield distribution in 240Pu(sf ) compared to that of 242Pu(sf ).

  12. Determination of the multiplication factor and its bias by the {sup 252}Cf-source technique: A method for code benchmarking with subcritical configurations

    SciTech Connect

    Perez, R.B.; Valentine, T.E.; Mihalczo, J.T.; Mattingly, J.K.

    1997-08-01

    A brief discussion of the Cf-252 source driven method for subcritical measurements serves as an introduction to the concept and use of the spectral ratio, {Gamma}. It has also been shown that the Monte Carlo calculation of spectral densities and effective multiplication factors have as a common denominator the transport propagator. This commonality follows from the fact that the Neumann series expansion of the propagator lends itself to the Monte Carlo method. On this basis a linear relationship between the spectral ratio and the effective multiplication factor has been shown. This relationship demonstrates the ability of subcritical measurements of the ratio of spectral densities to validate transport theory methods and cross sections.

  13. Dual-fission chamber and neutron beam characterization for fission product yield measurements using monoenergetic neutrons

    NASA Astrophysics Data System (ADS)

    Bhatia, C.; Fallin, B.; Gooden, M. E.; Howell, C. R.; Kelley, J. H.; Tornow, W.; Arnold, C. W.; Bond, E. M.; Bredeweg, T. A.; Fowler, M. M.; Moody, W. A.; Rundberg, R. S.; Rusev, G.; Vieira, D. J.; Wilhelmy, J. B.; Becker, J. A.; Macri, R.; Ryan, C.; Sheets, S. A.; Stoyer, M. A.; Tonchev, A. P.

    2014-09-01

    A program has been initiated to measure the energy dependence of selected high-yield fission products used in the analysis of nuclear test data. We present out initial work of neutron activation using a dual-fission chamber with quasi-monoenergetic neutrons and gamma-counting method. Quasi-monoenergetic neutrons of energies from 0.5 to 15 MeV using the TUNL 10 MV FM tandem to provide high-precision and self-consistent measurements of fission product yields (FPY). The final FPY results will be coupled with theoretical analysis to provide a more fundamental understanding of the fission process. To accomplish this goal, we have developed and tested a set of dual-fission ionization chambers to provide an accurate determination of the number of fissions occurring in a thick target located in the middle plane of the chamber assembly. Details of the fission chamber and its performance are presented along with neutron beam production and characterization. Also presented are studies on the background issues associated with room-return and off-energy neutron production. We show that the off-energy neutron contribution can be significant, but correctable, while room-return neutron background levels contribute less than <1% to the fission signal.

  14. A new design of fission detector for prompt fission neutron investigation

    NASA Astrophysics Data System (ADS)

    Zeynalov, Sh.; Zeynalova, O.; Nazarenko, M. A.; Hambsch, F.-J.; Oberstedt, S.

    2012-10-01

    In this work we report recent achievements in design of twin back-to-back ionization chamber (TIC) for fission fragment (FF) mass and kinetic energy spectroscopy. Correlated FF kinetic energies, their masses and the angle of the fission axes in 3D Cartesian coordinates can be determined from analysis of the heights and shapes of the pulses induced by the fission fragments on the anodes of TIC. Anodes of TIC were designed as consisting of isolated strips each having independent electronic circuitry and special multi-channel pulse processing apparatus. Mathematical algorithms were provided along with formulae derived for fission axis angles determination. It was shown how the point of fission fragments origin on the target plane may be determined using the same measured data. The last feature made the TIC a rather powerful tool for prompt fission neutron (PFN) emission investigation in event by event analysis of individual fission reactions from non point fissile source. Position sensitive neutron induced fission detector for neutron imaging applications with both thermal and low energy neutrons was found as another possible implementation of the designed TIC.

  15. Event-by-event fission simulation code, generates complete fission events

    2013-04-01

    FREYA is a computer code that generates complete fission events. The output includes the energy and momentum of these final state particles: fission products, prompt neutrons and prompt photons. The version of FREYA that is to be released is a module for MCNP6.

  16. Inhibition of peroxisome fission, but not mitochondrial fission, increases yeast chronological lifespan.

    PubMed

    Lefevre, Sophie D; Kumar, Sanjeev; van der Klei, Ida J

    2015-01-01

    Mitochondria are key players in aging and cell death. It has been suggested that mitochondrial fragmentation, mediated by the Dnm1/Fis1 organelle fission machinery, stimulates aging and cell death. This was based on the observation that Saccharomyces cerevisiae Δdnm1 and Δfis1 mutants show an enhanced lifespan and increased resistance to cell death inducers. However, the Dnm1/Fis1 fission machinery is also required for peroxisome division. Here we analyzed the significance of peroxisome fission in yeast chronological lifespan, using yeast strains in which fission of mitochondria was selectively blocked. Our data indicate that the lifespan extension caused by deletion of FIS1 is mainly due to a defect in peroxisome fission and not caused by a block in mitochondrial fragmentation. These observations are underlined by our observation that deletion of FIS1 does not lead to lifespan extension in yeast peroxisome deficient mutant cells.

  17. Fission Surface Power Technology Development Update

    NASA Technical Reports Server (NTRS)

    Palac, Donald T.; Mason, Lee S.; Houts, Michael G.; Harlow, Scott

    2011-01-01

    Power is a critical consideration in planning exploration of the surfaces of the Moon, Mars, and places beyond. Nuclear power is an important option, especially for locations in the solar system where sunlight is limited or environmental conditions are challenging (e.g., extreme cold, dust storms). NASA and the Department of Energy are maintaining the option for fission surface power for the Moon and Mars by developing and demonstrating technology for a fission surface power system. The Fission Surface Power Systems project has focused on subscale component and subsystem demonstrations to address the feasibility of a low-risk, low-cost approach to space nuclear power for surface missions. Laboratory demonstrations of the liquid metal pump, reactor control drum drive, power conversion, heat rejection, and power management and distribution technologies have validated that the fundamental characteristics and performance of these components and subsystems are consistent with a Fission Surface Power preliminary reference concept. In addition, subscale versions of a non-nuclear reactor simulator, using electric resistance heating in place of the reactor fuel, have been built and operated with liquid metal sodium-potassium and helium/xenon gas heat transfer loops, demonstrating the viability of establishing system-level performance and characteristics of fission surface power technologies without requiring a nuclear reactor. While some component and subsystem testing will continue through 2011 and beyond, the results to date provide sufficient confidence to proceed with system level technology readiness demonstration. To demonstrate the system level readiness of fission surface power in an operationally relevant environment (the primary goal of the Fission Surface Power Systems project), a full scale, 1/4 power Technology Demonstration Unit (TDU) is under development. The TDU will consist of a non-nuclear reactor simulator, a sodium-potassium heat transfer loop, a power

  18. Options For Development of Space Fission Propulsion Systems

    NASA Technical Reports Server (NTRS)

    Houta, Mike; VanDyke, Melissa; Godfroy, Tom; Pedersen, Kevin; Martin, James; Dickens, Ricky; Salvail, Pat; Hrbud, Ivana; Rodgers, Stephen L. (Technical Monitor)

    2001-01-01

    Fission technology can enable rapid, affordable access to any point in the solar system. Potential fission-based transportation options include high specific power continuous impulse propulsion systems and bimodal nuclear thermal rockets. Despite their tremendous potential for enhancing or enabling deep space and planetary missions, to date space fission system have only been used in Earth orbit. The first step towards utilizing advanced fission propulsion systems is development of a safe, near-term, affordable fission system that can enhance or enable near-term missions of interest. An evolutionary approach for developing space fission propulsion systems is proposed.

  19. Correlation of recent fission product release data

    SciTech Connect

    Kress, T.S.; Lorenz, R.A.; Nakamura, T.; Osborne, M.F.

    1989-01-01

    For the calculation of source terms associated with severe accidents, it is necessary to model the release of fission products from fuel as it heats and melts. Perhaps the most definitive model for fission product release is that of the FASTGRASS computer code developed at Argonne National Laboratory. There is persuasive evidence that these processes, as well as additional chemical and gas phase mass transport processes, are important in the release of fission products from fuel. Nevertheless, it has been found convenient to have simplified fission product release correlations that may not be as definitive as models like FASTGRASS but which attempt in some simple way to capture the essence of the mechanisms. One of the most widely used such correlation is called CORSOR-M which is the present fission product/aerosol release model used in the NRC Source Term Code Package. CORSOR has been criticized as having too much uncertainty in the calculated releases and as not accurately reproducing some experimental data. It is currently believed that these discrepancies between CORSOR and the more recent data have resulted because of the better time resolution of the more recent data compared to the data base that went into the CORSOR correlation. This document discusses a simple correlational model for use in connection with NUREG risk uncertainty exercises. 8 refs., 4 figs., 1 tab.

  20. Spontaneous subgaleal aerocele.

    PubMed

    Ibe, M O N; Onu, D O; Igwe, N N

    2014-01-01

    Apart from reporting about a case of spontaneous subgaleal aerocele this paper looks at the possible causes and management also. A 35-year-old Igbo-Nigerian female, about 4 weeks post-natal, with a 10-month old steadily and gradually enlarging mass around the back of her head, including both temporal regions was referred to us. Plain skull radiographs showed air in this mass. Needle puncture produced air leading to immediate and complete flattening of the lesion. A few hours after this procedure while still in the hospital premises, she had generalized convulsions, for which she was hospitalized and treated. With no further attacks, her request for discharge the following day was granted. At the next visit, 7 days later, there was a re-accumulation, which was treated the same way as previously and with the same result. She has not reported back since then, though she was advised to visit us again in 7 day-time. This lesion should be considered when masses on the head are presented. Our health institutions should have adequate investigative facilities.

  1. Spontaneous breaking of supersymmetry

    SciTech Connect

    Zumino, B.

    1981-12-01

    There has been recently a revival of interest in supersymmetric gauge theories, stimulated by the hope that supersymmetry might help in clarifying some of the questions which remain unanswered in the so called Grand Unified Theories and in particular the gauge hierarchy problem. In a Grand Unified Theory one has two widely different mass scales: the unification mass M approx. = 10/sup 15/GeV at which the unification group (e.g. SU(5)) breaks down to SU(3) x SU(2) x U(1) and the mass ..mu.. approx. = 100 GeV at which SU(2) x U(1) is broken down to the U(1) of electromagnetism. There is at present no theoretical understanding of the extreme smallness of the ratio ..mu../M of these two numbers. This is the gauge hierarchy problem. This lecture attempts to review the various mechanisms for spontaneous supersymmetry breaking in gauge theories. Most of the discussions are concerned with the tree approximation, but what is presently known about radiative correction is also reviewed.

  2. Fission enhanced diffusion of uranium in zirconia

    NASA Astrophysics Data System (ADS)

    Bérerd, N.; Chevarier, A.; Moncoffre, N.; Sainsot, Ph.; Faust, H.; Catalette, H.

    2005-11-01

    This paper deals with the comparison between thermal and Fission Enhanced Diffusion (FED) of uranium into zirconia, representative of the inner face of cladding tubes. The experiments under irradiation are performed at the Institut Laue Langevin (ILL) in Grenoble using the Lohengrin spectrometer. A thin 235UO2 layer in direct contact with an oxidised zirconium foil is irradiated in the ILL high flux reactor. The fission product flux is about 1011 ions cm-2 s-1 and the target temperature is measured by an IR pyrometer. A model is proposed to deduce an apparent uranium diffusion coefficient in zirconia from the energy distribution broadening of two selected fission products. It is found to be equal to 10-15 cm2 s-1 at 480 °C and compared to uranium thermal diffusion data in ZrO2 in the same pressure and temperature conditions. The FED results are analysed in comparison with literature data.

  3. Solar vs. Fission Surface Power for Mars

    NASA Technical Reports Server (NTRS)

    Rucker, Michelle A.; Oleson, Steve; George, Pat; Landis, Geoffrey A.; Fincannon, James; Bogner, Amee; Jones, Robert E.; Turnbull, Elizabeth; Martini, Michael C.; Gyekenyesi, John Z.; Colozza, Anthony J.; Schmitz, Paul C.; Packard, Thomas W.

    2016-01-01

    A multi-discipline team of experts from the National Aeronautics and Space Administration (NASA) developed Mars surface power system point design solutions for two conceptual missions. The primary goal of this study was to compare the relative merits of solar- versus fission-powered versions of each surface mission. First, the team compared three different solar power options against a fission power system concept for a sub-scale, uncrewed demonstration mission. The 4.5 meter (m) diameter pathfinder lander's primary mission would be to demonstrate Mars entry, descent, and landing techniques. Once on the Martian surface, the lander's In Situ Resource Utilization (ISRU) payload would demonstrate liquid oxygen propellant production using atmospheric resources. For the purpose of this exercise, location was assumed to be at the Martian equator. The three solar concepts considered included a system that only operated during daylight hours (at roughly half the daily propellant production rate of a round-the-clock fission design), a battery-augmented system that operated through the night (matching the fission concept's propellant production rate), and a system that operated only during daylight, but at a higher rate (again, matching the fission concept's propellant production rate). Including 30% mass growth allowance, total payload masses for the three solar concepts ranged from 1,116 to 2,396 kg, versus the 2,686 kg fission power scheme. However, solar power masses are expected to approach or exceed the fission payload mass at landing sites further from the equator, making landing site selection a key driver in the final power system decision. The team also noted that detailed reliability analysis should be performed on daytime-only solar power schemes to assess potential issues with frequent ISRU system on/off cycling. Next, the team developed a solar-powered point design solution for a conceptual four-crew, 500-day surface mission consisting of up to four landers per

  4. Lunar surface fission power supplies: Radiation issues

    SciTech Connect

    Houts, M.G.; Lee, S.K.

    1994-07-01

    A lunar space fission power supply shield that uses a combination of lunar regolith and materials brought from earth may be optimal for early lunar outposts and bases. This type of shield can be designed such that the fission power supply does not have to be moved from its landing configuration, minimizing handling and required equipment on the lunar surface. Mechanisms for removing heat from the lunar regolith are built into the shield, and can be tested on earth. Regolith activation is greatly reduced compared with a shield that uses only regolith, and it is possible to keep the thermal conditions of the fission power supply close to these seen in free space. For a well designed shield, the additional mass required to be brought fro earth should be less than 1000 kg. Detailed radiation transport calculations confirm the feasibility of such a shield.

  5. Molecular control of fission yeast cytokinesis.

    PubMed

    Rincon, Sergio A; Paoletti, Anne

    2016-05-01

    Cytokinesis gives rise to two independent daughter cells at the end of the cell division cycle. The fission yeast Schizosaccharomyces pombe has emerged as one of the most powerful systems to understand how cytokinesis is controlled molecularly. Like in most eukaryotes, fission yeast cytokinesis depends on an acto-myosin based contractile ring that assembles at the division site under the control of spatial cues that integrate information on cell geometry and the position of the mitotic apparatus. Cytokinetic events are also tightly coordinated with nuclear division by the cell cycle machinery. These spatial and temporal regulations ensure an equal cleavage of the cytoplasm and an accurate segregation of the genetic material in daughter cells. Although this model system has specificities, the basic mechanisms of contractile ring assembly and function deciphered in fission yeast are highly valuable to understand how cytokinesis is controlled in other organisms that rely on a contractile ring for cell division.

  6. Solution-processable singlet fission photovoltaic devices.

    PubMed

    Yang, Le; Tabachnyk, Maxim; Bayliss, Sam L; Böhm, Marcus L; Broch, Katharina; Greenham, Neil C; Friend, Richard H; Ehrler, Bruno

    2015-01-14

    We demonstrate the successful incorporation of a solution-processable singlet fission material, 6,13-bis(triisopropylsilylethynyl)pentacene (TIPS-pentacene), into photovoltaic devices. TIPS-pentacene rapidly converts high-energy singlet excitons into pairs of triplet excitons via singlet fission, potentially doubling the photocurrent from high-energy photons. Low-energy photons are captured by small-bandgap electron-accepting lead chalcogenide nanocrystals. This is the first solution-processable singlet fission system that performs with substantial efficiency with maximum power conversion efficiencies exceeding 4.8%, and external quantum efficiencies of up to 60% in the TIPS-pentacene absorption range. With PbSe nanocrystal of suitable bandgap, its internal quantum efficiency reaches 170 ± 30%.

  7. METHOD OF MAKING JACKETED FISSIONABLE SLUG

    DOEpatents

    Young, G.J.; Ohlinger, L.A.

    1959-02-10

    BS>A method is described for fabricating a jacketed fissionable body or slug to provide an effective leak-proof seal between the jacket and the end closure. A housing for the fissionable slug is first formed and then tinned on the interior. The fissionable slug is coated on its exterior surface with the same material used to tin the interior of the housing. The coated slug is then inserted into the housing. A disc shaped end closure for the housing, coated with the tinning material, is inserted into the open end of the housing while the tinning material is still liquid. The end of the housing is then swaged into good contact with the periphery of the closure.

  8. Low-mass fission detector for the fission neutron spectrum measurement

    SciTech Connect

    Wu, C Y; Henderson, R; Gostic, J; Haight, R C; Lee, H Y

    2010-10-20

    For the fission neutron spectrum measurement, the neutron energy is determined in a time-of-flight experiment by the time difference between the fission event and detection of the neutron. Therefore, the neutron energy resolution is directly determined by the time resolution of both neutron and fission detectors. For the fission detection, the detector needs not only a good timing response but also the tolerance of radiation damage and high {alpha}-decay rate. A parallel-plate avalanche counter (PPAC) has many advantages for the detection of heavy charged particles such as fission fragments. These include fast timing, resistance to radiation damage, and tolerance of high counting rate. A PPAC also can be tuned to be insensitive to particles, which is important for experiments with - emitting actinides. Therefore, a PPAC is an ideal detector for experiments requiring a fast and clean trigger for fission. In the following sections, the description will be given for the design and performance of a new low-mass PPAC for the fission-neutron spectrum measurements at LANL.

  9. Study on fission blanket fuel cycling of a fusion-fission hybrid energy generation system

    NASA Astrophysics Data System (ADS)

    Zhou, Z.; Yang, Y.; Xu, H.

    2011-10-01

    This paper presents a preliminary study on neutron physics characteristics of a light water cooled fission blanket for a new type subcritical fusion-fission hybrid reactor aiming at electric power generation with low technical limits of fission fuel. The major objective is to study the fission fuel cycling performance in the blanket, which may possess significant impacts on the feasibility of the new concept of fusion-fission hybrid reactor with a high energy gain (M) and tritium breeding ratio (TBR). The COUPLE2 code developed by the Institute of Nuclear and New Energy Technology of Tsinghua University is employed to simulate the neutronic behaviour in the blanket. COUPLE2 combines the particle transport code MCNPX with the fuel depletion code ORIGEN2. The code calculation results show that soft neutron spectrum can yield M > 20 while maintaining TBR >1.15 and the conversion ratio of fissile materials CR > 1 in a reasonably long refuelling cycle (>five years). The preliminary results also indicate that it is rather promising to design a high-performance light water cooled fission blanket of fusion-fission hybrid reactor for electric power generation by directly loading natural or depleted uranium if an ITER-scale tokamak fusion neutron source is achievable.

  10. Total and spontaneous fission half-lives for uranium and plutonium nuclides

    SciTech Connect

    Holden, N.E.

    1985-01-01

    Several reported experiments have been reanalyzed and recommended values are presented for /sup 232,233,234,235,236,238/U and for /sup 236,238,239,240,241,242,244/Pu. These values improve upon previous preliminary estimates of both the half-lives and the standard deviations. 120 refs., 23 tabs. (WRF)

  11. Solar Versus Fission Surface Power for Mars

    NASA Technical Reports Server (NTRS)

    Rucker, Michelle A.; Oleson, Steve; George, Pat; Landis, Geoffrey A.; Fincannon, James; Bogner, Amee; Jones, Robert E.; Turnbull, Elizabeth; McNatt, Jeremiah; Martini, Michael C.; Gyekenyesi, John Z.; Colozza, Anthony J.; Schmitz, Paul C.; Packard, Thomas W.

    2016-01-01

    A multi-discipline team of experts from the National Aeronautics and Space Administration (NASA) developed Mars surface power system point design solutions for two conceptual missions to Mars using In-situ resource utilization (ISRU). The primary goal of this study was to compare the relative merits of solar- versus fission-powered versions of each surface mission. First, the team compared three different solar-power options against a fission power system concept for a sub-scale, uncrewed demonstration mission. This “pathfinder” design utilized a 4.5 meter diameter lander. Its primary mission would be to demonstrate Mars entry, descent, and landing techniques. Once on the Martian surface, the lander’s ISRU payload would demonstrate liquid oxygen propellant production from atmospheric resources. For the purpose of this exercise, location was assumed to be at the Martian equator. The three solar concepts considered included a system that only operated during daylight hours (at roughly half the daily propellant production rate of a round-the-clock fission design), a battery-augmented system that operated through the night (matching the fission concept’s propellant production rate), and a system that operated only during daylight, but at a higher rate (again, matching the fission concept’s propellant production rate). Including 30% mass growth allowance, total payload masses for the three solar concepts ranged from 1,128 to 2,425 kg, versus the 2,751 kg fission power scheme. However, solar power masses increase as landing sites are selected further from the equator, making landing site selection a key driver in the final power system decision. The team also noted that detailed reliability analysis should be performed on daytime-only solar power schemes to assess potential issues with frequent ISRU system on/off cycling.

  12. Decay and Fission Hindrance of Two- and Four-Quasiparticle K Isomers in ^{254}Rf.

    PubMed

    David, H M; Chen, J; Seweryniak, D; Kondev, F G; Gates, J M; Gregorich, K E; Ahmad, I; Albers, M; Alcorta, M; Back, B B; Baartman, B; Bertone, P F; Bernstein, L A; Campbell, C M; Carpenter, M P; Chiara, C J; Clark, R M; Cromaz, M; Doherty, D T; Dracoulis, G D; Esker, N E; Fallon, P; Gothe, O R; Greene, J P; Greenlees, P T; Hartley, D J; Hauschild, K; Hoffman, C R; Hota, S S; Janssens, R V F; Khoo, T L; Konki, J; Kwarsick, J T; Lauritsen, T; Macchiavelli, A O; Mudder, P R; Nair, C; Qiu, Y; Rissanen, J; Rogers, A M; Ruotsalainen, P; Savard, G; Stolze, S; Wiens, A; Zhu, S

    2015-09-25

    Two isomers decaying by electromagnetic transitions with half-lives of 4.7(1.1) and 247(73) μs have been discovered in the heavy ^{254}Rf nucleus. The observation of the shorter-lived isomer was made possible by a novel application of a digital data acquisition system. The isomers were interpreted as the K^{π}=8^{-}, ν^{2}(7/2^{+}[624],9/2^{-}[734]) two-quasineutron and the K^{π}=16^{+}, 8^{-}ν^{2}(7/2^{+}[624],9/2^{-}[734])⊗8^{-}π^{2}(7/2^{-}[514],9/2^{+}[624]) four-quasiparticle configurations, respectively. Surprisingly, the lifetime of the two-quasiparticle isomer is more than 4 orders of magnitude shorter than what has been observed for analogous isomers in the lighter N=150 isotones. The four-quasiparticle isomer is longer lived than the ^{254}Rf ground state that decays exclusively by spontaneous fission with a half-life of 23.2(1.1) μs. The absence of sizable fission branches from either of the isomers implies unprecedented fission hindrance relative to the ground state.

  13. Dynamic fission instability of dissipative protoplanets

    NASA Technical Reports Server (NTRS)

    Boss, A. P.; Mizuno, H.

    1985-01-01

    Analytical and numerical approaches are taken to consider if a rapidly rotating, viscous protoearth would have lost mass by a fission process and thereby given birth to the moon. The fast rotation is assumed as the source of the instability in the dissipative liquid protoearth. Governing hydrodynamic equations are defined for the evolution of the protoearth. Account is taken of viscous dissipation, the pressure equation of state for the atmospheric material sent on a ballistic trajectory, and the effective viscosity. The results indicate that dynamic fission was probably not the process by which the protomoon came into existence.

  14. In-beam Fission Study at JAEA

    NASA Astrophysics Data System (ADS)

    Nishio, Katsuhisa

    2013-12-01

    Fission fragment mass distributions were measured in heavy-ion induced fissions using 238U target nucleus. The measured mass distributions changed drastically with incident energy. The results are explained by a change of the ratio between fusion and quasifission with nuclear orientation. A calculation based on a fluctuation dissipation model reproduced the mass distributions and their incident energy dependence. Fusion probability was determined in the analysis. Evaporation residue cross sections were calculated with a statistical model in the reactions of 30Si + 238U and 34S + 238U using the obtained fusion probability in the entrance channel. The results agree with the measured cross sections for seaborgium and hassium isotopes.

  15. Italian hybrid and fission reactors scenario analysis

    NASA Astrophysics Data System (ADS)

    Ciotti, M.; Manzano, J.; Sepielli, M.

    2012-06-01

    Italy is a country where a long tradition of studies both in the fission and fusion field is consolidated; nevertheless a strong public opinion concerned with the destination of the Spent Nuclear Fuel hinders the development of nuclear power. The possibility to a severe reduction of the NSF mass generated from a fleet of nuclear reactors employing an hypothetical fusionfission hybrid reactor has been investigated in the Italian framework. The possibility to produce nuclear fuel for the fission nuclear reactors with the hybrid reactor was analyzed too.

  16. Uranium arc fission reactor for space propulsion

    NASA Astrophysics Data System (ADS)

    Watanabe, Yoichi; Maya, Isaac; Vitali, Juan; Appelbaum, Jacob; Schneider, Richard T.

    Combining the proven technology of solid core reactors with uranium arc confinement and non-equilibrium ionization by fission fragments can lead to an attractive propulsion system which has a higher specific impulse than a solid core propulsion system and higher thrust than an electric propulsion system. A preliminary study indicates that a system with 300 MW of fission power can achieve a gas exhaust velocity of 18,000 m/sec and a thrust of 10,000 Newtons utilizing a magnetohydrodynamic generator and accelerator. An experimental program is underway to examine the major mass and energy transfer issues.

  17. Uranium arc fission reactor for space propulsion

    NASA Astrophysics Data System (ADS)

    Watanabe, Yoichi; Maya, Isaac; Vitali, Juan; Appelbaum, Jacob; Schneider, Richard T.

    1991-01-01

    Combining the proven technology of solid core reactors with uranium arc confinement and non-equilibrium ionization by fission fragments can lead to an attractive propulsion system which has a higher specific impulse than a solid core propulsion system and higher thrust than an electric propulsion systems. A preliminary study indicates that a system with 300 MW of fission power can achieve a gas exhaust velocity of 18,000 m/sec and a thrust of 10,000 Newtons utilizing a magnetohydrodynamic generator and accelerator. An experimental program is underway to examine the major mass and energy transfer issues.

  18. Dynamic fission instability of dissipative protoplanets

    NASA Astrophysics Data System (ADS)

    Boss, A. P.; Mizuno, H.

    1985-07-01

    Analytical and numerical approaches are taken to consider if a rapidly rotating, viscous protoearth would have lost mass by a fission process and thereby given birth to the moon. The fast rotation is assumed as the source of the instability in the dissipative liquid protoearth. Governing hydrodynamic equations are defined for the evolution of the protoearth. Account is taken of viscous dissipation, the pressure equation of state for the atmospheric material sent on a ballistic trajectory, and the effective viscosity. The results indicate that dynamic fission was probably not the process by which the protomoon came into existence.

  19. Three's company: the fission yeast actin cytoskeleton.

    PubMed

    Kovar, David R; Sirotkin, Vladimir; Lord, Matthew

    2011-03-01

    How the actin cytoskeleton assembles into different structures to drive diverse cellular processes is a fundamental cell biological question. In addition to orchestrating the appropriate combination of regulators and actin-binding proteins, different actin-based structures must insulate themselves from one another to maintain specificity within a crowded cytoplasm. Actin specification is particularly challenging in complex eukaryotes where a multitude of protein isoforms and actin structures operate within the same cell. Fission yeast Schizosaccharomyces pombe possesses a single actin isoform that functions in three distinct structures throughout the cell cycle. In this review we explore recent studies in fission yeast that help unravel how different actin structures operate in cells.

  20. Uncertainty Quantification on Prompt Fission Neutrons Spectra

    SciTech Connect

    Talou, P. Madland, D.G.; Kawano, T.

    2008-12-15

    Uncertainties in the evaluated prompt fission neutrons spectra present in ENDF/B-VII.0 are assessed in the framework of the Los Alamos model. The methodology used to quantify the uncertainties on an evaluated spectrum is introduced. We also briefly review the Los Alamos model and single out the parameters that have the largest influence on the calculated results. Using a Kalman filter, experimental data and uncertainties are introduced to constrain model parameters, and construct an evaluated covariance matrix for the prompt neutrons spectrum. Preliminary results are shown in the case of neutron-induced fission of {sup 235}U from thermal up to 15 MeV incident energies.

  1. Italian hybrid and fission reactors scenario analysis

    SciTech Connect

    Ciotti, M.; Manzano, J.; Sepielli, M.

    2012-06-19

    Italy is a country where a long tradition of studies both in the fission and fusion field is consolidated; nevertheless a strong public opinion concerned with the destination of the Spent Nuclear Fuel hinders the development of nuclear power. The possibility to a severe reduction of the NSF mass generated from a fleet of nuclear reactors employing an hypothetical fusionfission hybrid reactor has been investigated in the Italian framework. The possibility to produce nuclear fuel for the fission nuclear reactors with the hybrid reactor was analyzed too.

  2. The development of an optimized neutron proportional counter for fission spectra

    NASA Astrophysics Data System (ADS)

    Millett, Marshall Geary

    Some of the materials used to make a nuclear weapon (isotopes of uranium and plutonium) are inherently unstable and undergo radioactive decay, including spontaneous fission. This spontaneous fission results in the generation of high energy neutrons that will likely escape the nuclear device. Since neutrons in the fission energy range are not common in the environment and are relatively difficult to shield, the detection of fission neutrons is useful for arms control applications such as illicit material detection or nuclear weapon treaty verification. Although neutron detectors are currently available (and utilized) for such applications, they either are excessively heavy or have low counting efficiency. This research effort comprises the development of an optimized neutron detector and is unique in that both weight and counting efficiency have been optimized for the detection of fission neutrons. The difficulty of this optimization process lies in the fact that detector weight and counting efficiency are mutually dependent. This dissertation presents the research and conclusions that lead to the optimized design, including calculations, computer modeling, model validation, and laboratory verification. Computer modeling was conducted using the MCNP (Monte Carlo N Particle) neutron transport code. For model validation and laboratory verification, a special cylindrical detector was built, called the "USNA detector," which allowed for the changing of fill gas composition and pressure as well as moderator thickness. Using this detector, experimental data were collected in order to test the effectiveness of various fill gas combinations and to provide a benchmark for the computer code. After validating computer generated results, the development of an optimized detector design proceeded by use of computer modeling. This dissertation first presents background information and initial design considerations used to determine detector and moderator candidates. The

  3. Exergonic and Spontaneous Production of Radicals through Beryllium Bonds.

    PubMed

    Brea, Oriana; Alkorta, Ibon; Mó, Otilia; Yáñez, Manuel; Elguero, José; Corral, Inés

    2016-07-18

    High-level ab initio calculations show that the formation of radicals, by the homolytic bond fission of Y-R (Y=F, OH, NH2 ; R=CH3 , NH2 , OH, F, SiH3 , PH2 , SH, Cl, NO) bonds is dramatically favored by the association of the molecule with BeX2 (X=H and Cl) derivatives. This finding is a consequence of two concomitant effects, the significant activation of the Y-R bond after the formation of the beryllium bond, and the huge stabilization of the F(.) (OH(.) , NH2 (.) ) radical upon BeX2 attachment. In those cases where R is an electronegative group, the formation of the radicals is not only exergonic, but spontaneous.

  4. Exergonic and Spontaneous Production of Radicals through Beryllium Bonds.

    PubMed

    Brea, Oriana; Alkorta, Ibon; Mó, Otilia; Yáñez, Manuel; Elguero, José; Corral, Inés

    2016-07-18

    High-level ab initio calculations show that the formation of radicals, by the homolytic bond fission of Y-R (Y=F, OH, NH2 ; R=CH3 , NH2 , OH, F, SiH3 , PH2 , SH, Cl, NO) bonds is dramatically favored by the association of the molecule with BeX2 (X=H and Cl) derivatives. This finding is a consequence of two concomitant effects, the significant activation of the Y-R bond after the formation of the beryllium bond, and the huge stabilization of the F(.) (OH(.) , NH2 (.) ) radical upon BeX2 attachment. In those cases where R is an electronegative group, the formation of the radicals is not only exergonic, but spontaneous. PMID:27308835

  5. Spontaneous resolution of subfoveal perfluorocarbon

    PubMed Central

    Oellers, Patrick; Charkoudian, Leon D; Hahn, Paul

    2015-01-01

    Perfluorocarbon liquids (PFCL) have transformed the surgical approach to complex retinal detachments, but their use can be complicated by subretinal retention. Migration of peripherally located subretinal PFCL towards the fovea is well established, but spontaneous resolution of subfoveal PFCL without surgical evacuation or displacement has rarely been described. We present a case of a large single retained subfoveal PFCL droplet following vitrectomy with membrane peeling, inferior relaxing retinectomy, and silicone oil tamponade that demonstrated spontaneous resolution 3 weeks postoperatively, with subsequent anatomic and visual improvement. No residual subretinal PFCL was noted, and we hypothesize that the PFCL droplet spontaneously extruded through a transient hole created in the thinned retina overlying the droplet, which subsequently closed spontaneously. Further understanding of the mechanisms of PFCL migration and resolution may facilitate improved treatments for this complication. PMID:25834389

  6. Fission barriers in a macroscopic-microscopic model

    SciTech Connect

    Dobrowolski, A.; Pomorski, K.; Bartel, J.

    2007-02-15

    In the framework of the macroscopic-microscopic model, this study investigates fission barriers in the region of actinide nuclei. A very effective four-dimensional shape parametrization for fissioning nuclei is proposed. Taking, in particular, the left-right mass asymmetric and nonaxial shapes into account is demonstrated to have a substantial effect on fission barrier heights. The influence of proton versus neutron deformation differences on the potential energy landscape of fissioning nuclei is also discussed.

  7. New results on the ternary fission of 243Cm

    NASA Astrophysics Data System (ADS)

    Heyse, J.; Wagemans, C.; Vermote, S.; Serot, O.; Geltenbort, P.; Soldner, T.; Van Gils, J.

    2005-11-01

    Ternary fission is an important source of He and tritium gas in nuclear reactors and used fuel elements. Therefore a systematic study of the ternary fission yields for 4He and tritons (t) is being performed. In recent years the influence of the excitation energy of the fissioning nucleus on the triton emission probability (t/B) has been investigated for different Cm and Cf isotopes. In this paper we report on new results on the neutron induced fission of 243Cm.

  8. Structure of matter, radioactivity, and nuclear fission. Volume 3

    SciTech Connect

    Not Available

    1986-01-01

    Subject matter includes structure of matter (what is matter, forces holding atoms together, visualizing the atom, the chemical elements, atomic symbols, isotopes, radiation from the atom), radioactivity (what holds the nucleus together, can one element change into another element, radiation from the nucleus, half-life, chart of the nuclides), and nuclear fission (nuclear energy release, the fission process, where does fission energy go, radiation and radioactivity resulting from fission).

  9. Development and Utilization of Space Fission Power Systems

    NASA Technical Reports Server (NTRS)

    Houts, Michael; Mason, Lee S.; Palac, Donald T.; Harlow, Scott E.

    2008-01-01

    Space fission power systems could enable advanced civilian space missions. Terrestrially, thousands of fission systems have been operated since 1942. In addition, the US flew a space fission system in 1965, and the former Soviet Union flew 33 such systems prior to the end of the Cold War. Modern design and development practices, coupled with 65 years of experience with terrestrial reactors, could enable the affordable development of space fission power systems for near-term planetary surface applications.

  10. Development and Utilization of Space Fission Power Systems

    NASA Technical Reports Server (NTRS)

    Houts, Michael G.; Mason, Lee S.; Palac, Donald T.; Harlow, Scott E.

    2009-01-01

    Space fission power systems could enable advanced civilian space missions. Terrestrially, thousands of fission systems have been operated since 1942. In addition, the US flew a space fission system in 1965, and the former Soviet Union flew 33 such systems prior to the end of the Cold War. Modern design and development practices, coupled with 65 years of experience with terrestrial reactors, could enable the affordable development of space fission power systems for near-term planetary surface applications.

  11. Optimally moderated nuclear fission reactor and fuel source therefor

    DOEpatents

    Ougouag, Abderrafi M.; Terry, William K.; Gougar, Hans D.

    2008-07-22

    An improved nuclear fission reactor of the continuous fueling type involves determining an asymptotic equilibrium state for the nuclear fission reactor and providing the reactor with a moderator-to-fuel ratio that is optimally moderated for the asymptotic equilibrium state of the nuclear fission reactor; the fuel-to-moderator ratio allowing the nuclear fission reactor to be substantially continuously operated in an optimally moderated state.

  12. Fission Matrix Capability for MCNP Monte Carlo

    SciTech Connect

    Carney, Sean E.; Brown, Forrest B.; Kiedrowski, Brian C.; Martin, William R.

    2012-09-05

    In a Monte Carlo criticality calculation, before the tallying of quantities can begin, a converged fission source (the fundamental eigenvector of the fission kernel) is required. Tallies of interest may include powers, absorption rates, leakage rates, or the multiplication factor (the fundamental eigenvalue of the fission kernel, k{sub eff}). Just as in the power iteration method of linear algebra, if the dominance ratio (the ratio of the first and zeroth eigenvalues) is high, many iterations of neutron history simulations are required to isolate the fundamental mode of the problem. Optically large systems have large dominance ratios, and systems containing poor neutron communication between regions are also slow to converge. The fission matrix method, implemented into MCNP[1], addresses these problems. When Monte Carlo random walk from a source is executed, the fission kernel is stochastically applied to the source. Random numbers are used for: distances to collision, reaction types, scattering physics, fission reactions, etc. This method is used because the fission kernel is a complex, 7-dimensional operator that is not explicitly known. Deterministic methods use approximations/discretization in energy, space, and direction to the kernel. Consequently, they are faster. Monte Carlo directly simulates the physics, which necessitates the use of random sampling. Because of this statistical noise, common convergence acceleration methods used in deterministic methods do not work. In the fission matrix method, we are using the random walk information not only to build the next-iteration fission source, but also a spatially-averaged fission kernel. Just like in deterministic methods, this involves approximation and discretization. The approximation is the tallying of the spatially-discretized fission kernel with an incorrect fission source. We address this by making the spatial mesh fine enough that this error is negligible. As a consequence of discretization we get a

  13. Fission Product Sorptivity in Graphite

    SciTech Connect

    Tompson, Jr., Robert V.; Loyalka, Sudarshan; Ghosh, Tushar; Viswanath, Dabir; Walton, Kyle; Haffner, Robert

    2015-04-01

    Both adsorption and absorption (sorption) of fission product (FP) gases on/into graphite are issues of interest in very high temperature reactors (VHTRs). In the original proposal, we proposed to use packed beds of graphite particles to measure sorption at a variety of temperatures and to use an electrodynamic balance (EDB) to measure sorption onto single graphite particles (a few μm in diameter) at room temperature. The use of packed beds at elevated temperature is not an issue. However, the TPOC requested revision of this initial proposal to included single particle measurements at elevated temperatures up to 1100 °C. To accommodate the desire of NEUP to extend the single particle EDB measurements to elevated temperatures it was necessary to significantly revise the plan and the budget. These revisions were approved. In the EDB method, we levitate a single graphite particle (the size, surface characteristics, morphology, purity, and composition of the particle can be varied) or agglomerate in the balance and measure the sorption of species by observing the changes in mass. This process involves the use of an electron stepping technique to measure the total charge on a particle which, in conjunction with the measured suspension voltages for the particle, allows for determinations of mass and, hence, of mass changes which then correspond to measurements of sorption. Accommodating elevated temperatures with this type of system required a significant system redesign and required additional time that ultimately was not available. These constraints also meant that the grant had to focus on fewer species as a result. Overall, the extension of the original proposed single particle work to elevated temperatures added greatly to the complexity of the proposed project and added greatly to the time that would eventually be required as well. This means that the bulk of the experimental progress was made using the packed bed sorption systems. Only being able to recruit one

  14. Spontaneous Activity in Crustacean Neurons

    PubMed Central

    Preston, James B.; Kennedy, Donald

    1962-01-01

    Single units which discharged with regular spontaneous rhythms without intentional stimulation were observed in the ventral nerve cord by intracellular recording close to the sixth abdominal ganglion. These units were divided into two groups: group A units in which interspike intervals varied less than 10 msec.; group B units in which interspike intervals varied within a range of 10 to 30 msec. Group A units maintained "constant" interspike intervals and could not be discharged by sensory inputs, while the majority of group B units could be discharged by appropriate sensory nerve stimulation. Both group A and B units discharged to direct stimulation when the stimulating and recording electrodes were placed in the same ganglionic intersegment, and directly evoked single spikes reset the spontaneous rhythm. In group B units, presynaptic volleys reset the spontaneous rhythm of some units; but in others, synaptically evoked spikes were interpolated within the spontaneous rhythm without resetting. The phenomenon of enhancement could also be demonstrated in spontaneously active units as a result of repetitive stimulation. It is concluded that endogenous pacemaker activity is responsible for much of the regular spontaneous firing observed in crayfish central neurons, and that interaction of evoked responses with such pacemaker sites can produce a variety of effects dependent upon the anatomical relationships between pacemaker and synaptic regions. PMID:14488667

  15. Fission measurements with PPAC detectors using a coincidence technique

    SciTech Connect

    Paradela, C.; Duran, I.; Tarrio, D.; Audouin, L.; Tassan-Got, L.; Stephan, C.

    2011-07-01

    A fission detection setup based on Parallel Plate Avalanche Counters (PPAC) has been constructed and used at the CERN n-TOF facility. The setup takes advantage of the coincidence detection of both fission fragments to discriminate the background reactions produced by high energy neutrons and it allows obtaining neutron-induced fission cross section up to 1 GeV. (authors)

  16. Thermodynamics and Spontaneity

    NASA Astrophysics Data System (ADS)

    Ochs, Raymond S.

    1996-10-01

    Despite the importance of thermodynamics as the foundation of chemistry, most students emerge from introductory courses with only a dim understanding of this subject. Generally students recognize that the information is significant, yet do not assimilate it into later studies, especially in applied fields such as biology and biochemistry. A clear sense of the problem is reflected in a number of other contributions to this Journal (e.g., 1 - 6). Most (1 - 4, 6) recommend increased rigor in derivation of equations. This may appeal to students in advanced courses in chemical thermodynamics, but not to most. A few other suggestions are to introduce the subject earlier in general chemistry courses (2) or to provide innovative ways to visualize reaction changes (3). I suggest that the problem lies at another level entirely: the meanings of the terms are not clear. Recently, MacNeal (7) introduced the concept of mathsemantics, the joining of mathematics with a deep understanding of the sense (semantics) in which it operates. For example, the author argues that not only can we add apples and oranges (yielding total fruit), but that anything less than such a synthesis is trivial. Mathematics is hard, not because of the actual mathematical part of the problem but because of the semantics. As discussed thoroughly by Weinburg (8), the very names we affix to ideas dominate how we think about them. A similar reorientation would benefit chemical education. By way of example, the word "spontaneous" is widely used in thermodynamics, presumably because the word is familiar and assists understanding of this subject. In the following, I will provide evidence that this word has contributed more to the obfuscation of chemical ideas than it has helped elucidate them. Literature Cited 1. Redlich, O. J. Chem. Educ. 1975, 52, 374 - 376. 2. Bergquist, W.; Heikkinen, H. J. Chem. Educ. 1990, 67, 1000 - 1003. 3. Macomber, R. S. J. Chem. Educ. 1994, 71, 311 - 312. 4. Sanchez, K. S.; Vergenz, R

  17. Delayed neutrons in fission of polonium isotopes

    SciTech Connect

    Ramazanov, R.; Urikbaev, Z.S.; Maksyutenko, B.P.; Ignat'ev, S.V.

    1988-06-01

    A strong difference is found in the relative yields of delayed neutrons in the production of compound nuclei of polonium isotopes in reactions in which bismuth and lead are bombarded by various charged particles. The effect can be partially explained by the different lengths of the ..beta..-decay chains of the light and heavy fission products.

  18. Propagation of a constant velocity fission wave

    NASA Astrophysics Data System (ADS)

    Deinert, Mark

    2011-10-01

    The ideal nuclear fuel cycle would require no enrichment, minimize the need fresh uranium, and produce few, if any, transuranic elements. Importantly, the latter goal would be met without the reprocessing. For purely physical reasons, no reactor system or fuel cycle can meet all of these objectives. However, a traveling-wave reactor, if feasible, could come remarkably close. The concept is simple: a large cylinder of natural (or depleted) uranium is subjected to a fast neutron source at one end, the neutrons would transmute the uranium downstream and produce plutonium. If the conditions were right, a self-sustaining fission wave would form, producing yet more neutrons which would breed more plutonium and leave behind little more than short-lived fission products. Numerical studies have shown that fission waves of this type are also possible. We have derived an exact solution for the propagation velocity of a fission wave through fertile material. The results show that these waves fall into a class of traveling wave phenomena that have been encountered in other systems. The solution places a strict conditions on the shapes of the flux, diffusive, and reactive profiles that would be required for such a phenomenon to persist. The results are confirmed numerically.

  19. Cutting fluid for machining fissionable materials

    SciTech Connect

    Duerksen, W.K.; Googin, J.M.; Napier, B. Jr.

    1982-01-28

    The present invention is directed to a cutting fluid for machining fissionable material. The cutting fluid is formed of glycol, water and a boron compound in an adequate concentration for effective neutron attenuation so as to inhibit criticality incidents during machining.

  20. Liquid uranium alloy-helium fission reactor

    DOEpatents

    Minkov, V.

    1984-06-13

    This invention describes a nuclear fission reactor which has a core vessel and at least one tandem heat exchanger vessel coupled therewith across upper and lower passages to define a closed flow loop. Nuclear fuel such as a uranium alloy in its liquid phase fills these vessels and flow passages. Solid control elements in the reactor core vessel are adapted to be adjusted relative to one another to control fission reaction of the liquid fuel therein. Moderator elements in the other vessel and flow passages preclude fission reaction therein. An inert gas such as helium is bubbled upwardly through the heat exchanger vessel operable to move the liquid fuel upwardly therein and unidirectionally around the closed loop and downwardly through the core vessel. This helium gas is further directed to heat conversion means outside of the reactor vessels to utilize the heat from the fission reaction to generate useful output. The nuclear fuel operates in the 1200 to 1800/sup 0/C range, and even higher to 2500/sup 0/C.