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Sample records for 3h 4he 16o

  1. Contributions of excited {sup 6}Li and {sup 7}Li nuclei to the production of {sup 4}He+{sup 2}H and {sup 4}He+{sup 3}H systems in {sup 16}O{sub p} collisions at a momentum of 3.25 GeV/c per nucleon

    SciTech Connect

    Olimov, K.; Glagolev, V. V.; Gulamov, K. G.; Lutpullaev, S. L.; Kurbanov, A. R.; Olimov, A. K.; Petrov, V. I.; Yuldashev, A. A.

    2013-07-15

    New experimental data on the cross sections for the yield of excited {sup 6}Li* and {sup 7}Li* nuclei and on their contributions to the production of {sup 4}He + {sup 2}H and {sup 4}He+{sup 3}H light dinuclear systems in {sup 16}O{sub p} collisions at a momentumof 3.25 A GeV/c per nucleon are presented.

  2. Direct measurement of the 4He (12C, 16O) γ reaction cross section near stellar energies

    NASA Astrophysics Data System (ADS)

    Sagara, Kenshi

    2014-09-01

    The 12C+4He-->16O + γ reaction is one of the key reactions in stellar He-burning, but its total cross section at stellar energy (Ecm = 0.3 MeV) has not been measured yet, in spite of many experiments made in the world for about a half century. At Kyushu University Tandem accelerator Laboratory (KUTL), we have been making direct measurement of the 4He (12C, 16O) γ total cross section below Ecm = 2.4 MeV for about 20 years. We have measured the total cross section at Ecm = 2.4, 1.5 and 1.2 MeV. Now we are preparing to measure the cross section at 1.0 MeV. The direct measurement was made from Ecm = 5 MeV down to 1.9 MeV at Ruhr University, Bochum. We use a pulsed 12C beam and a windowless 4He target, and detect all the 16O recoils in a charge state. A usually continuum 12C beam from our tandem accelerator is pulsed by a pre-buncher, a main buncher, and a beam chopper. Our tandem accelerator was designed to be used at the acceleration voltage of 6-10 MV. For the 4He (12C, 16O) γ experiment we need to use it at 1.3-1.8 MV where beam transmission is very low, then we have invented an acceleration-deceleration method for the tandem accelerator. We have developed a blow-in windowless He target based on an original idea. To separate 16O recoils from the 12C beam, we developed a recoil-mass separator. To reject 12C backgrounds, we developed a long-time chopper, and an ionization chamber. Now, we are preparing to measure time-of-flight of 16O recoils and 12C backgrounds. Many original instruments and the experimental results will be presented. Finally we discuss what are necessary for future direct measurement of the 4He (12C, 16O) γ total cross section below 1.0 MeV, down to 0.7 MeV. A dynamitron accelerator and hard-working researchers may be inevitable. The 12C+4He-->16O + γ reaction is one of the key reactions in stellar He-burning, but its total cross section at stellar energy (Ecm = 0.3 MeV) has not been measured yet, in spite of many experiments made in the world

  3. Spin polarization effects in the /sup 3/H(d,n)/sup 4/He fusion reaction

    SciTech Connect

    Conzett, H.E.; Rioux, C.

    1985-06-01

    A recent investigation has shown that the /sup 3/H(d,n)/sup 4/He fusion reaction rate could be enhanced by a factor of 3/2 if the fusion plasma consisted of both polarized deuterons and tritons, forming exclusively the channel-spin S = 3/2, J = 3/2/sup +/ state. This result follows simply from the statistical weights of the quartet S = 3/2 and doublet S = 1/2 initial states, with the assumption of the single J = 3/2/sup +/ reaction amplitude. Since, with a small but nonzero J = 1/2/sup +/ amplitude, the maximum enhancement of the reaction occurs at the peak of the J = 3/2/sup +/ resonance, corresponding to a deuteron lab energy of 107 keV, it is of obvious interest to know what the enhancement would be at the lower energies that are typical of fusion plasmas. We are able to address this question by extending earlier calculations which gave the values of all of the spin-polarization observables at this J = 3/2/sup +/ resonance in both the /sup 3/H(d,n)/sup 4/He and the /sup 3/He(d,p)/sup 4/He reactions.

  4. Barshay-Temmer test for the 4He( overlined, 3He) 3H reaction

    NASA Astrophysics Data System (ADS)

    Bruno, M.; Cannata, F.; D'agostino, M.; Fiandri, M. L.; Herman, M.; Hofmann, H. M.; Vuaridel, B.; Grüebler, W.; König, V.; Schmelzbach, P. A.; Elsener, K.

    1989-09-01

    The mechanisms of isospin violation in the reaction 4He( overlined, 3He) 3H is studied, in the framework of a microscopic model. To describe realistically the intermediate 6Li nucleus and the fragment states we use the refined resonating group model (RRGM). A detailed analysis of the matrix elements responsible for the asymmetry of cross sections and vector analyzing powers is presented. The isospin violation is found typically of the order of 5-10% and arises mainly from coupling to intermediate "5 + 1" structures in a two-step mechanism. The agreement with the experimental data is fair.

  5. Ab initio many-body calculations of the (3)H(d,n)(4)He and (3)He(d,p)(4)He fusion reactions.

    PubMed

    Navrátil, Petr; Quaglioni, Sofia

    2012-01-27

    We apply the ab initio no-core shell model combined with the resonating-group method approach to calculate the cross sections of the (3)H(d,n)(4)He and (3)He(d,p)(4)He fusion reactions. These are important reactions for the big bang nucleosynthesis and the future of energy generation on Earth. Starting from a selected similarity-transformed chiral nucleon-nucleon interaction that accurately describes two-nucleon data, we performed many-body calculations that predict the S factor of both reactions. Virtual three-body breakup effects are obtained by including excited pseudostates of the deuteron in the calculation. Our results are in satisfactory agreement with experimental data and pave the way for microscopic investigations of polarization and electron-screening effects, of the (3)H(d,γn)(4)He bremsstrahlung and other reactions relevant to fusion research. PMID:22400830

  6. Polarization Transfer in 4He(e-vector,e[prime]p-vector)3H

    SciTech Connect

    Michael Paolone

    2007-10-01

    Polarization transfer in quasi-elastic nucleon knockout is sensitive to the properties of the nucleon in the nuclear medium, including possible modification of the nucleon form factor and/or spinor. In our recently completed experiment E03-104 at Jefferson Lab we measured the proton recoil polarization in the 4He(e-vector,e[prime]p-vector)3H reaction at a Q2 of 0.8 (GeV/c)2 and 1.3 (GeV/c)2 with unprecedented precision. These data complement earlier data between 0.4 and 2.6 (GeV/c)2 from both Mainz and Jefferson Lab, in which the measured ratio of polarization-transfer coefficients differs from a fully relativistic DWIA calculation. Preliminary results hint at a possible unexpected Q2 dependence in the polarization transfer coefficient ratio. Final analysis will help constrain FSI models

  7. Medium Modifications from {sup 4}He(e-vector,e'p-vector){sup 3}H

    SciTech Connect

    Malace, S.; Paolone, M.; Strauch, S.

    2008-10-13

    Polarization transfer in quasi-elastic nucleon knockout is sensitive to the properties of the nucleon in the nuclear medium, including possible modification of the nucleon form factor and/or spinor. In our recently completed experiment E03-104 at Jefferson Lab we measured the proton recoil polarization in the {sup 4}He(e-vector,e'p-vector){sup 3}H reaction at a Q{sup 2} of 0.8 (GeV/c){sup 2} and 1.3 (GeV/c){sup 2} with unprecedented precision. These data complement earlier data between 0.4 and 2.6 (GeV/c){sup 2} from both Mainz and Jefferson Lab. The measured ratio of polarization-transfer coefficients differs from a fully relativistic calculation, favoring either the inclusion of a medium modification of the proton form factors predicted by a quark-meson coupling model or strong charge-exchange final-state interactions. The measured induced polarizations agree well with the fully relativistic calculation and indicate that these strong final-state interactions may not be applicable.

  8. Ab Initio Many-Body Calculations Of n-3H, n-4He, p-3,4He, And n-10Be Scattering

    SciTech Connect

    Quaglioni, S; Navratil, P

    2008-03-26

    We develop a new ab initio many-body approach capable of describing simultaneously both bound and scattering states in light nuclei, by combining the resonating-group method with the use of realistic interactions, and a microscopic and consistent description of the nucleon clusters. This approach preserves translational symmetry and Pauli principle. We present phase shifts for neutron scattering on {sup 3}H, {sup 4}He and {sup 10}Be and proton scattering on {sup 3,4}He, using realistic nucleon-nucleon potentials. Our A = 4 scattering results are compared to earlier ab initio calculations. We demonstrate that a proper treatment of the coupling to the n-{sup 10}Be continuum is essential to explain the parity-inverted ground state in {sup 11}Be.

  9. The 4He(e,e'p)3H Reaction at Jlab

    SciTech Connect

    Bodo Reitz

    2003-05-01

    In the recent experiment E97-111 at Jefferson Lab the unseparated cross section for the (e,e{prime}p) reaction on {sup 4}He was measured at recoil momenta up to 530 MeV/c. In the plane-wave impulse approximation, many calculations predict a sharp minimum in the cross section for recoil momenta around 450 MeV/c and show that its location is sensitive to the short-range part of the internucleon potential. However, reaction dynamic effects such as final-state interactions and meson-exchange currents can obscure such a minimum. To distinguish and study these effects data were taken at several different kinematic points. The preliminary results of the experiment are presented and compared to recent model calculations.

  10. Comparative study of dose distributions and cell survival fractions for 1H, 4He, 12C and 16O beams using Geant4 and Microdosimetric Kinetic model

    NASA Astrophysics Data System (ADS)

    Burigo, Lucas; Pshenichnov, Igor; Mishustin, Igor; Bleicher, Marcus

    2015-04-01

    Depth and radial dose profiles for therapeutic 1H, 4He, 12C and 16O beams are calculated using the Geant4-based Monte Carlo model for Heavy-Ion Therapy (MCHIT). 4He and 16O ions are presented as alternative options to 1H and 12C broadly used for ion-beam cancer therapy. Biological dose profiles and survival fractions of cells are estimated using the modified Microdosimetric Kinetic model. Depth distributions of cell survival of healthy tissues, assuming 10% and 50% survival of tumor cells, are calculated for 6 cm SOBPs at two tumor depths and for different tissues radiosensitivities. It is found that the optimal ion choice depends on (i) depth of the tumor, (ii) dose levels and (iii) the contrast of radiosensitivities of tumor and surrounding healthy tissues. Our results indicate that 12C and 16O ions are more appropriate to spare healthy tissues in the case of a more radioresistant tumor at moderate depths. On the other hand, a sensitive tumor surrounded by more resistant tissues can be better treated with 1H and 4He ions. In general, 4He beam is found to be a good candidate for therapy. It better spares healthy tissues in all considered cases compared to 1H. Besides, the dose conformation is improved for deep-seated tumors compared to 1H, and the damage to surrounding healthy tissues is reduced compared to heavier ions due to the lower impact of nuclear fragmentation. No definite advantages of 16O with respect to 12C ions are found in this study.

  11. A precise extraction of the induced polarization in the 4He(e,e'p)3H reaction

    SciTech Connect

    S.P. Malace, M. Paolone, S. Strauch

    2011-01-01

    We measured with unprecedented precision the induced polarization Py in 4He(e,e'p)3H at Q^2 = 0.8 (GeV/c)^2 and 1.3 (GeV/c)^2. The induced polarization is indicative of reaction-mechanism effects beyond the impulse approximation. Our results are in agreement with a relativistic distorted-wave impulse approximation calculation but are over-estimated by a calculation with strong charge-exchange effects. Our data are used to constrain the strength of the spin independent charge-exchange term in the latter calculation.

  12. Polarization Transfer in {sup 4}He(e-vector,e{sup '}p-vector){sup 3}H

    SciTech Connect

    Paolone, Michael

    2007-10-26

    Polarization transfer in quasi-elastic nucleon knockout is sensitive to the properties of the nucleon in the nuclear medium, including possible modification of the nucleon form factor and/or spinor. In our recently completed experiment E03-104 at Jefferson Lab we measured the proton recoil polarization in the {sup 4}He(e-vector,e{sup '}p-vector){sup 3}H reaction at a Q{sup 2} of 0.8 (GeV/c){sup 2} and 1.3 (GeV/c){sup 2} with unprecedented precision. These data complement earlier data between 0.4 and 2.6 (GeV/c){sup 2} from both Mainz and Jefferson Lab, in which the measured ratio of polarization-transfer coefficients differs from a fully relativistic DWIA calculation. Preliminary results hint at a possible unexpected Q{sup 2} dependence in the polarization transfer coefficient ratio. Final analysis will help constrain FSI models.

  13. Direct Measurement of the 4He(12C, 16O)γ Total Cross Section Near Stellar Energies

    NASA Astrophysics Data System (ADS)

    Fujita, Kunihiro; Yamaguchi, Hiroyuki; Ban, Tadahiko; Hamamoto, Kenichi; Narikiyo, Yoshihiro; Tao, Nariaki; Sagara, Kenshi

    2015-05-01

    A cross section measurement employing a direct 16O detection method for the reaction energies from Ecm = 2.4 to 0.7 MeV is planned at Kyushu University Tandem Laboratory (KUTL). To perform this experiment and to obtain quantitative information about the cross section to within an error of 10%, we have developed several instruments, including a blow-in type windowless gas target, a recoil mass separator and a RF-deflector. The measurements at Ecm = 2.4 and 1.5 MeV have been performed with these instruments. For measuring at Ecm < 1.2 MeV, a hybrid detector employing both, an ionization chamber and a silicon detector was developed to reduce the carbon backgrounds more efficiently. The oxygen ions were clearly separated from carbon background by using the energy deposit in the ionization chamber. Experiment of Ecm = 1.2 MeV was performed and the cross section was obtained.

  14. Ab initio study of {sup 2}H(d,{gamma}){sup 4}He, {sup 2}H(d,p){sup 3}H, and {sup 2}H(d,n){sup 4}He reactions and the tensor force

    SciTech Connect

    Arai, K.; Aoyama, S.; Suzuki, Y.; Descouvemont, P.; Baye, D.

    2012-11-12

    The {sup 2}H(d,p){sup 3}H, {sup 2}H(d,n){sup 3}He, and {sup 2}H(d,{gamma}){sup 4}He reactions at low energies are studied with realistic nucleon-nucleon interactions in an ab initio approach. The obtained astrophysical S-factors are all in very good agreement with experiment. The most important channels for both transfer and radiative capture are all found to dominate thanks to the tensor force.

  15. Search for sup 3 H, sub 3 He, and sub 4 He in D sub 2 -loaded titanium

    SciTech Connect

    Clarke, W.B.; Clarke, R.M. )

    1992-03-01

    In this paper a search is described for {sup 3}He, {sup 4}He, and tritium produced when D{sub 2} is absorbed by titanium sponge, or released when titanium deuteride is heated. The D{sub 2} is prepared from pre-nuclear-era D{sub 2}O, which has a tritium/deuterium (T/D) ratio of 1.8 {times} 10{sup {minus}15}. Two reservoirs of titanium sponge in a vacuum system attached to the inlet line of a mass spectrometer are heated to allow rapid transfer of D{sub 2} from one sponge to the other. Significant amounts of {sup 3}He and {sup 4}He are released only after the deuterium content is increased to reach TiD{sub 1.5} in one sponge. Then {sup 3}He and {sup 4}He are decreased as the D{sub 2} is transferred back and forth. When the titanium is loaded to a composition of TiD{sub 2.0}, {sup 3}He and {sup 4}He increase during the next two transfers, then decrease. When the D{sub 2} is replaced by H{sub 2}, then D{sub 2}-H{sub 2} (1:1), {sup 3}He and {sup 4}He decrease steadily, indicating that the transfer process causes partial release of {sup 3}He and {sup 4}He trapped in the titanium.

  16. The {sup 3}He(e,e'p){sup 2}H and {sup 4}He(e,e'p){sup 3}H reactions at high momentum transfer

    SciTech Connect

    Ford, William P.; Schiavilla, Rocco; Van Orden, J. W.

    2014-03-01

    We present updated calculations for observables in the processes {sup 3}He(e,e'p){sup 2}H, {sup 4}He(e,e'p){sup 3}H and {sup 4}He(e-vector, e'p-vector){sup 3}H. This update entails the implementation of improved nucleon-nucleon (NN) amplitudes to describe final state interactions (FSI) within a Glauber approximation and includes full spin-isospin dependence in the profile operator. In addition, an optical potential, which has also been updated since previous work, is utilized to treat FSI for the {sup 4}He(e,e'p){sup 3}H and {sup 4}He(e-vector, e'p-vector){sup 3}H reactions. The calculations are compared with experimental data and show good agreement between theory and experiment. Comparisons are made between the various approximations in the Glauber treatment, including model dependence due to the NN scattering amplitudes, rescattering contributions, and spin dependence. We also analyze the validity of the Glauber approximation at the kinematics the data is available, by comparing to the results obtained with the optical potential.

  17. Photodisintegration cross section of the reaction (4)He(γ,p)(3)H between 22 and 30 MeV.

    PubMed

    Raut, R; Tornow, W; Ahmed, M W; Crowell, A S; Kelley, J H; Rusev, G; Stave, S C; Tonchev, A P

    2012-01-27

    The two-body photodisintegration cross section of (4)He into a proton and triton was measured with monoenergetic photon beams in 0.5 MeV energy steps between 22 and 30 MeV. High-pressure (4)He-Xe gas scintillators of various (4)He/Xe ratios served as targets and detectors. Pure Xe gas scintillators were used for background studies. A NaI detector together with a plastic scintillator paddle was employed for determining the incident photon flux. Our comprehensive data set follows the trend of the theoretical calculations of the Trento group very well, although our data are consistently lower in magnitude by about 5%. However, they differ significantly from the majority of the previous data, especially from the recent data of Shima et al. The latter data had put into question the validity of theoretical approaches used to calculate core-collapse supernova explosions and big-bang nucleosynthesis abundances of certain light nuclei. PMID:22400829

  18. Estimating the groundwater residence time in eskers of the Amos region, northern Quebec by 3H-3He and (U-Th/4He) methods

    NASA Astrophysics Data System (ADS)

    Boucher, Christine; Berthot, Laureline; Pinti, Daniele Luigi; Larocque, Marie; Cloutier, Vincent; Blanchette, Daniel; Castro, Maria Clara; Hall, Chris M.

    2013-04-01

    An esker is a long winding ridge of stratified sand and gravel. The eskers of the Amos region (Abitibi-Témiscamingue, Québec) that were deposited during the last deglaciation, are known to be aquifers containing drinking water of exceptional quality. Yet little is known about their hydrologic regime and exchanges with other water sources. A better understanding of these systems is necessary to assess the vulnerability of these aquifers to contaminants and to implement a management plan for these resources. A multi-isotopic study of groundwater in the eskers of the Amos region (Saint-Mathieu-Berry, Barraute and Harricana moraine) was carried out in 2011-2012. Noble gas isotopes, together with major ions chemistry and stable isotopes were used to estimate the residence time of waters, to trace fluid flow paths and to determine the atmospheric temperature at the time of the recharge took place. Measured 3He/4He ratios were primarily used to identify mixing between different water types carrying distinct helium components. The 20Ne/4He vs. 3He/4He relationship shows that waters flowing into eskers have three helium components: atmospheric, tritiogenic 3He-rich and radiogenic 4He-rich. The measured 3He/4He ratios (R) normalized to the atmospheric one (R/Ra) varies between 0.224±0.012 and 1.849±0.036. Most radiogenic 4He-rich mineralized waters are those from fractured basement rocks of Archean age. Freshwater flowing into eskers show mixing between radiogenic helium and tritiogenic 3He. A clear relationship between the well depths, salinity and the 3He/4He ratios suggests that mixing occurs between these two groundwater bodies. Tritium measurements allow the calculation of 3H-3He ages varying from 6.7±1.3 yrs to 9.7±1.3 yrs for waters flowing through the Harricana moraine. Groundwater from Saint-Mathieu de Berry esker ranges from 11.0±2.1 yrs to 32.5±1.6 yrs. The 3H-3He ages plotted against the wells depth show a linear relationship for both, the Saint

  19. Polarization transfer in the 4He(e→,e'p→)3H reaction at Q2 = 0.8 and 1.3 (GeV/c)2

    DOE PAGES

    Michael Paolone; Malace, Simona P.

    2010-08-12

    Here, proton recoil polarization was measured in the quasielastic 4He(e→,e'p→)3H reaction at Q2 = 0.8 (GeV/c)2 and 1.3 (GeV/c)2 with unprecedented precision. The polarization-transfer coefficients are found to differ from those of the 1H(e→,e'p→) reaction, contradicting a relativistic distorted-wave approximation, and favoring either the inclusion of medium-modified proton form factors predicted by the quark-meson coupling model or a spin-dependent charge-exchange final-state interaction. For the first time, the polarization-transfer ratio is studied as a function of the virtuality of the proton.

  20. Polarization Transfer in the 4He(e→,e'p→)3H Reaction up to Q2=2.6 (GeV/c)2

    NASA Astrophysics Data System (ADS)

    Strauch, S.; Dieterich, S.; Aniol, K.; Annand, J.; Baker, O.; Bertozzi, W.; Boswell, M.; Brash, E.; Chai, Z.; Chen, J.-P.; Christy, M.; Chudakov, E.; Cochran, A.; de Leo, R.; Ent, R.; Epstein, M.; Finn, J.; Fissum, K.; Forest, T.; Frullani, S.; Garibaldi, F.; Gasparian, A.; Gayou, O.; Gilad, S.; Gilman, R.; Glashausser, C.; Gomez, J.; Gorbenko, V.; Gueye, P.; Hansen, J.; Higinbotham, D.; Hu, B.; Hyde-Wright, C.; Ireland, D.; Jackson, C.; de Jager, C.; Jiang, X.; Jones, C.; Jones, M.; Kellie, J.; Kelly, J.; Keppel, C.; Kumbartzki, G.; Kuss, M.; Lerose, J.; Livingston, K.; Liyanage, N.; Malov, S.; Margaziotis, D.; Meekins, D.; Michaels, R.; Mitchell, J.; Nanda, S.; Nappa, J.; Perdrisat, C.; Punjabi, V.; Ransome, R.; Roché, R.; Rosner, G.; Rvachev, M.; Sabatie, F.; Saha, A.; Sarty, A.; Udias, J.; Ulmer, P.; Urciuoli, G.; van den Brand, J.; Vignote, J.; Watts, D.; Weinstein, L.; Wijesooriya, K.; Wojtsekhowski, B.

    2003-07-01

    We have measured the proton recoil polarization in the 4He(e→ ,e'p→)4H reaction at Q2=0.5, 1.0, 1.6, and 2.6 (GeV/c)2. The measured ratio of polarization transfer coefficients differs from a fully relativistic calculation, favoring the inclusion of a medium modification of the proton form factors predicted by a quark-meson coupling model. In addition, the measured induced polarizations agree reasonably well with the fully relativistic calculation indicating that the treatment of final-state interactions is under control.

  1. Diffraction dissociation of {sup 7}Li and {sup 7}Be relativistic nuclei on proton targets through the {sup 3}H({sup 3}He)+{sup 4}He channels

    SciTech Connect

    Fetisov, V. N.

    2015-07-15

    For the fragmentation of {sup 7}Li and {sup 7}Be relativistic nuclei (with momenta of, respectively, P = 3 GeV/c and P = 1.6 GeV/c per nucleon) on proton targets through the {sup 3}H({sup 3}He) + {sup 4}He channels, the differential cross sections with respect to the momentum transfer Q to the fragments were calculated on the basis of the cluster version of Akhiezer–Glauber–Sitenko diffraction theory by employing the twobody cluster model for the {sup 7}Li ({sup 3}H + {sup 4}He) and {sup 7}Be ({sup 3}He + {sup 4}He) nuclei. These calculations, performed in the impulse approximation in the interaction of intranuclear clusters with the target nucleus, explained a strong suppression of the cross sections for reactions on protons at Q lower than 100 MeV/c and higher than 350 MeV/c and the observed irregularities in the behavior off the cross section for {sup 7}Li fragmentation on complex track-emulsion nuclei. Cross-section values close to their experimental counterparts were obtained upon setting the coefficient of two-body clustering in the {sup 7}Li and {sup 7}Be nuclei to k ≃ 0.7.

  2. Volumetric Properties of the Mixture Propenenitrile C3H3N + C7H16O Heptan-1-ol (VMSD1212, LB4921_V)

    NASA Astrophysics Data System (ADS)

    Cibulka, I.; Fontaine, J.-C.; Sosnkowska-Kehiaian, K.; Kehiaian, H. V.

    This document is part of Subvolume C 'Binary Liquid Systems of Nonelectrolytes III' of Volume 26 'Heats of Mixing, Vapor-Liquid Equilibrium, and Volumetric Properties of Mixtures and Solutions' of Landolt-Börnstein Group IV 'Physical Chemistry'. It contains the Chapter 'Volumetric Properties of the Mixture Propenenitrile C3H3N + C7H16O Heptan-1-ol (VMSD1212, LB4921_V)' providing data by calculation of molar excess volume from low-pressure density measurements at variable mole fraction and constant temperature.

  3. Volumetric Properties of the Mixture Propenenitrile C3H3N + C7H16O Heptan-1-ol (VMSD1211, LB4553_V)

    NASA Astrophysics Data System (ADS)

    Cibulka, I.; Fontaine, J.-C.; Sosnkowska-Kehiaian, K.; Kehiaian, H. V.

    This document is part of Subvolume C 'Binary Liquid Systems of Nonelectrolytes III' of Volume 26 'Heats of Mixing, Vapor-Liquid Equilibrium, and Volumetric Properties of Mixtures and Solutions' of Landolt-Börnstein Group IV 'Physical Chemistry'. It contains the Chapter 'Volumetric Properties of the Mixture Propenenitrile C3H3N + C7H16O Heptan-1-ol (VMSD1211, LB4553_V)' providing data from direct low-pressure dilatometric measurement of molar excess volume at variable mole fraction and constant temperature.

  4. Volumetric Properties of the Mixture Propenenitrile C3H3N + C7H16O Heptan-1-ol (VMSD1511, LB4929_V)

    NASA Astrophysics Data System (ADS)

    Cibulka, I.; Fontaine, J.-C.; Sosnkowska-Kehiaian, K.; Kehiaian, H. V.

    This document is part of Subvolume C 'Binary Liquid Systems of Nonelectrolytes III' of Volume 26 'Heats of Mixing, Vapor-Liquid Equilibrium, and Volumetric Properties of Mixtures and Solutions' of Landolt-Börnstein Group IV 'Physical Chemistry'. It contains the Chapter 'Volumetric Properties of the Mixture Propenenitrile C3H3N + C7H16O Heptan-1-ol (VMSD1511, LB4929_V)' providing data from direct measurement of low-pressure thermodynamic speed of sound at variable mole fraction and constant temperature, in the single-phase region(s).

  5. Volumetric Properties of the Mixture Propenenitrile C3H3N + C7H16O Heptan-1-ol (VMSD1111, LB4914_V)

    NASA Astrophysics Data System (ADS)

    Cibulka, I.; Fontaine, J.-C.; Sosnkowska-Kehiaian, K.; Kehiaian, H. V.

    This document is part of Subvolume C 'Binary Liquid Systems of Nonelectrolytes III' of Volume 26 'Heats of Mixing, Vapor-Liquid Equilibrium, and Volumetric Properties of Mixtures and Solutions' of Landolt-Börnstein Group IV 'Physical Chemistry'. It contains the Chapter 'Volumetric Properties of the Mixture Propenenitrile C3H3N + C7H16O Heptan-1-ol (VMSD1111, LB4914_V)' providing data from direct low-pressure measurement of mass density at variable mole fraction and constant temperature, in the single-phase region(s).

  6. Method for determination of {sup 18}O/{sup 16}O and {sup 2}H/{sup 1}H ratios and {sup 3}H (tritium) concentrations of xylem waters and subsurface waters using time-series sampling

    SciTech Connect

    1999-11-09

    This application describes a method for the determination of {sup 18}O/{sup 16}O and {sup 2}H/{sup 1}H ratios and {sup 3}H concentrations of xylem and subsurface waters using time-series sampling, insulating sampling chambers, and combined {sup 18}O/{sup 16}O, {sup 2}H/{sup 1}H and {sup 3}H concentration data on transpired water. The method involves collecting water samples transpired from living plants and correcting the measured isotopic compositions of oxygen ({sup 18}O/{sup 16}O) and hydrogen ({sup 2}H/{sup 1}H and/or {sup 3}H concentrations) to account for evaporative isotopic fractionation in the leafy material of the plant.

  7. Method for determination of .sup.18 O/.sup.16 O and .sup.2 H/.sup.1 H ratios and .sup.3 H (tritium) concentrations of xylem waters and subsurface waters using time series sampling

    DOEpatents

    Smith, Brian; Menchaca, Leticia

    1999-01-01

    A method for determination of .sup.18 O/.sup.16 O and .sup.2 H/.sup.1 H ratios and .sup.3 H concentrations of xylem and subsurface waters using time series sampling, insulating sampling chambers, and combined .sup.18 O/.sup.16 O, .sup.2 H/.sup.1 H and .sup.3 H concentration data on transpired water. The method involves collecting water samples transpired from living plants and correcting the measured isotopic compositions of oxygen (.sup.18 O/.sup.16 O) and hydrogen (.sup.2 H/.sup.1 H and/or .sup.3 H concentrations) to account for evaporative isotopic fractionation in the leafy material of the plant.

  8. Dose and dose averaged LET comparison of {sup 1}H, {sup 4}He, {sup 6}Li, {sup 8}Be, {sup 10}B, {sup 12}C, {sup 14}N, and {sup 16}O ion beams forming a spread-out Bragg peak

    SciTech Connect

    Kantemiris, I.; Karaiskos, P.; Papagiannis, P.; Angelopoulos, A.

    2011-12-15

    Purpose: Modern clinical accelerators are capable of producing ion beams from protons up to neon. This work compares the depth dose distribution and corresponding dose averaged linear energy transfer (LET) distribution, which is related to the biological effectiveness, for different ion beams ({sup 1}H, {sup 4}He, {sup 6}Li, {sup 8}Be, {sup 10}B, {sup 12}C, {sup 14}N, and {sup 16}O) using multi-energetic spectra in order to configure spread-out Bragg peaks (SOBP). Methods: Monte Carlo simulations were performed in order to configure a 5 cm SOBP at 8 cm depth in water for all the different ion beams. Physical dose and dose averaged LET distributions as a function of depth were then calculated and compared. The superposition of dose distribution of all ions is also presented for a two opposing fields configuration. Additional simulations were performed for {sup 12}C beams to investigate the dependence of dose and dose averaged LET distributions on target depth and size, as well as beam configuration. These included simulations for a 3 cm SOBP at 7, 10, and 13 cm depth in water, a 6 cm SOBP at 7 depth in water, and two opposing fields of 6 cm SOBP. Results: Alpha particles and protons present superior physical depth dose distributions relative to the rest of the beams studied. Dose averaged LET distributions results suggest higher biological effectiveness in the target volume for carbon, nitrogen and oxygen ions. This is coupled, however, with relatively high LET values--especially for the last two ion species--outside the SOBP where healthy tissue would be located. Dose averaged LET distributions for {sup 8}Be and {sup 10}B beams show that they could be attractive alternatives to {sup 12}C for the treatment of small, not deeply seated lesions. The potential therapeutic effect of different ion beams studied in this work depends on target volume and position, as well as the number of beams used. Conclusions: The optimization of beam modality for specific tumor cites

  9. Dipole Resonances in 4He

    SciTech Connect

    Matsumoto, E.; Nakayama, S.; Hayami, R.; Fushimi, K.; Kawasuso, H.; Yasuda, K.; Yamagata, T.; Akimune, H.; Ikemizu, H.; Fujiwara, M.; Yosoi, M.; Nakanishi, K.; Kawase, K.; Hashimoto, H.; Oota, T.; Sagara, K.; Kudoh, T.; Asaji, S.; Ishida, T.; Tanaka, M.

    2007-02-26

    We investigated the analogs of the giant dipole resonance (GDR) and spin-dipole resonance (SDR) of 4He by using the 4He(7Li,7Be) reaction at an incident energy of 455 MeV and at forward scattering angles. The {delta}S=0 and {delta}S=1 spectra for 4He were obtained by measuring the 0.43-MeV 7Be {gamma}-ray in coincidence with the scattered 7Be. From the {delta}S=0 and {delta}S=1 spectra thus obtained, the strength distributions of the GDR and SDR in 4He can be derived and the results are compared with the previous data.

  10. Condensate fraction in superfluid 4He

    NASA Astrophysics Data System (ADS)

    Olinto, A. C.

    1987-04-01

    Recently, a relationship between the chemical potential and the condensate fracton n0(T) has been derived for all temperatures in the superfluid region. An analysis of liquid 4He chemical-potential data yields n0(T=0)=0.062, and n0(T) is in excellent agreement with the empirical results of Svensson, Sears, and Griffin.

  11. sup 4 He- sup 4 He elastic scattering and variational wave functions

    SciTech Connect

    Usmani, A.A.; Ahmad, I. ); Usmani, Q.N. )

    1992-01-01

    We calculate differential cross sections for {sup 4}He-{sup 4}He elastic scattering at 4.32 GeV/{ital c} in the framework of Glauber multiple scattering theory using correlated variational wave functions as given by the two-nucleon Urbana {ital v}{sub 14} potential and the spin-isospin averaged Melfleit-Tjon force {ital V}. These wave functions are found to give fairly satisfactory results.

  12. Tortuosity of 4He Films on Aerogel

    SciTech Connect

    Ashton, C. E.; Golov, A. I.; Mulders, N.

    2006-09-07

    A torsional oscillator has been used to study the flow of liquid 4He through silica aerogel. The tortuosity and dissipation of the flow in the fractal aerogel environment has been measured, for both capillary condensed films and a fully saturated cell. The scaling of tortuosity as a function of filling fraction has been investigated. We compare the results of our 88%-porous aerogel to a 92%-porous sample where a transverse sound technique was used. Our more sensitive technique has reduced the scatter in both the frequency and dissipation data. Like in the previous transverse sound experiment, we find tortuosity as a function of filling fraction to scale with an exponent of {approx} -1.1. Further experiments are planned, to find the dependence of the exponent on the fractal dimension and porosity of aerogel.

  13. Superfluid 4He dynamics beyond quasiparticle excitations

    NASA Astrophysics Data System (ADS)

    Beauvois, K.; Campbell, C. E.; Dawidowski, J.; Fâk, B.; Godfrin, H.; Krotscheck, E.; Lauter, H.-J.; Lichtenegger, T.; Ollivier, J.; Sultan, A.

    2016-07-01

    The dynamics of superfluid 4He at and above the Landau quasiparticle regime is investigated by high-precision inelastic neutron scattering measurements of the dynamic structure factor. A highly structured response is observed above the familiar phonon-maxon-roton spectrum, characterized by sharp thresholds for phonon-phonon, maxon-roton, and roton-roton coupling processes. The experimental dynamic structure factor is compared to the calculation of the same physical quantity by a dynamic many-body theory including three-phonon processes self-consistently. The theory is found to provide a quantitative description of the dynamics of the correlated bosons for energies up to about three times that of the Landau quasiparticles.

  14. The ^3H(p,γ)^4He Reaction below 80 keV

    NASA Astrophysics Data System (ADS)

    Canon, R. S.; Kelley, J. H.; Nelson, S. O.; Schreiber, E. C.; Saburov, K.; Wulf, E. A.; Weller, H. R.; Prior, R. M.; Spraker, M.; Tilley, D. R.

    1999-10-01

    Significant advances in three body theory have resulted in excellent agreement with experimental radiative capture measurements(E. A. Wulf et al.), submitted to PRL. and emphasize the importance of MEC effects at energies below 100 keV(G. Schmid et al.), PRC 56, 2565 (1997).. Preliminary work has begun in applying these techniques to the four-body problem(A. Fonseca,W. Glöckle,A. Kievsky,H. Witala, (private communication).). In order to provide accurate experimental data for these forthcoming theoretical predictions, low energy polarized proton capture on tritium is being studied at TUNL. Preliminary results of these studies, which include a determination of the absolute cross section and measurements of the angular distributions of analyzing powers and cross sections, will be presented. Implications of these measurements will be discussed along with plans for future studies.

  15. Deeply Virtual Compton Scattering off 4He

    NASA Astrophysics Data System (ADS)

    Joosten, Sylvester; CLAS Collaboration

    2015-10-01

    The European Muon Collaboration (EMC) observed the first signs of a modification of the partonic structure of the nucleon when present in a nuclear medium. The precise nature of these effects, as well as their underlying cause, is yet to be determined. The generalized parton distribution (GPD) framework provides a powerful tool to study the partonic structure of nucleons inside a nucleus. Hard exclusive leptoproduction of a real photon off a nucleon, deeply virtual Compton scattering (DVCS), is presently considered the cleanest experimental access to the GPDs, through the Compton form factors (CFFs). This is especially the case for scattering off the spin-zero helium nucleus, where only a single CFF contributes to the process. The real and imaginary parts of this CFF can be constrained through the beam-spin asymmetry (BSA). We will present the first measurements of the DVCS process off 4He using the CEBAF 6 GeV polarized electron beam and the CLAS detector at JLab. The CLAS detector was supplemented with an inner electromagnetic calorimeter for photons produced at small angles, as well as a radial time projection chamber (RTPC) to detect low-energy recoil nuclei. This setup allowed for a clean measurement of the BSA in both the coherent and incoherent channels.

  16. Crystallization of 4He in aerogel via mass flow from surrounding solid 4He

    NASA Astrophysics Data System (ADS)

    Matsuda, H.; Ochi, A.; Isozaki, R.; Minami, S.; Nomura, R.; Pollanen, J.; Halperin, W. P.; Okuda, Y.

    2016-07-01

    The phase boundary between the quantum solid and the liquid phases of 4He is strongly modified in a porous material. However the phase diagram at very low temperatures remains unexplored. We have used a variable-volume experimental cell with optical access to visualize the crystallization of 4He in silica aerogels with independent control of the pressure and temperature. The onset of crystallization was investigated in two aerogel samples with differing porosity both by pressurization at constant temperature and by cooling at constant pressure. With isothermal pressurization we have established a low-temperature phase diagram for each aerogel, and we find that the equilibrium crystallization pressure is reduced with increasing aerogel porosity. Crystals also began to grow in the aerogel on cooling at fixed pressure below an onset temperature Tgrow. We found that below this temperature the crystallization rate increased with decreasing temperature. The aerogel in our cell was surrounded by bulk crystals of 4He , and surprisingly Tgrow was found to be widely distributed when the surrounding bulk crystals were repressurized. In this experimental arrangement, crystallization within the aerogel on cooling requires mass flow from these exterior bulk crystals and is strongly influenced by the disordered structure at the interface between the bulk solid and the helium within the aerogel.

  17. 4He abundances: Optical versus radio recombination line measurements

    NASA Astrophysics Data System (ADS)

    Balser, Dana S.; Rood, Robert T.; Bania, T. M.

    2010-04-01

    Accurate measurements of the 4He/H abundance ratio are important in constraining Big Bang nucleosynthesis, models of stellar and Galactic evolution, and H ii region physics. We discuss observations of radio recombination lines using the Green Bank Telescope toward a small sample of H ii regions and planetary nebulae. We report 4He/H abundance ratio differences as high as 15-20% between optical and ratio data that are difficult to reconcile. Using the H ii regions S206 and M17 we determine 4He production in the Galaxy to be dY/dZ = 1.71 ± 0.86.

  18. Sound velocity of liquid 4He in aerogel

    NASA Astrophysics Data System (ADS)

    Matsumoto, Koichi; Arai, Osamu; Okuda, Yuichi; Tajiri, Koji

    2000-07-01

    The sound velocity and attenuation of liquid 4He in 93.7% and 94.6% porosity aerogels were measured for a frequency of 10 MHz. The sound velocity in 93.7% aerogel was larger than that in bulk 4He, whereas that in 94.6% was smaller. A model of the aerogel- 4He composite gave satisfactory agreement with the dependence of the sound velocity on the temperature and the aerogel density. This shows that the normal fluid is clamped to aerogel strands, although the viscous penetration depth is comparable to the typical size of a void in the aerogel.

  19. Quantum Phase Transition of 4He Confined in Nanoporous Media

    SciTech Connect

    Shirahama, Keiya

    2006-09-07

    4He confined in nanoporous media is an excellent model system for studying a strongly correlated Bose liquid and solid in a confinement potential. We studied superfluidity and liquid-solid phase transition of 4He confined in a porous Gelsil glass that had nanopores 2.5 nm in diameter. The obtained pressure-temperature phase diagram is fairly unprecedented: the superfluid transition temperature approaches zero at 3.4 MPa, and the freezing pressure is enhanced by approximately 1 MPa from the bulk one. These features indicate that the confined 4He undergoes a superfluid-nonsuperfluid-solid quantum phase transition at zero temperature. The nonsuperfluid phase may be a localized Bose-condensed state in which global phase coherence is destroyed by a strong correlation between the 4He atoms or by a random potential.

  20. Significant structure theory applied to liquid 4He

    PubMed Central

    Ryoo, Ryong; Jhon, Mu Shik; Eyring, Henry

    1980-01-01

    The large kinetic zero-point motion of 4He molecules has been properly taken into account in the significant structure theory of liquids in order to describe the liquidity of liquid 4He. The Debye and the Bose-Einstein partition functions are used for the solid-like molecules of the normal fluid component and for the whole gas-like molecules, respectively. The solid-like molecules of the superfluid component are considered as ground state molecules without having positional degeneracies. The Bragg-Williams approximation of an order/disorder phase transition has been applied to the λ transition of liquid 4He. Thermodynamic and surface properties of liquid 4He have been calculated up to the critical point. The results are satisfactory when compared with the observed values. PMID:16592747

  1. Studies on the response of 3He and 4He proportional counters to monoenergetic fast neutrons

    NASA Astrophysics Data System (ADS)

    Manolopoulou, M.; Fragopoulou, M.; Stoulos, S.; Koukorava, C.; Spyrou, A.; Perdikakis, G.; Hashemi-Nezhad, S. R.; Zamani, M.

    2006-06-01

    Two helium filled proportional counters ( 3He and 4He) were studied to establish the optimum operating conditions when these counters are used for fast neutron measurements, as well as to examine the linearity of the pulse height with neutron energy. The detectors were irradiated with mono-energetic neutrons in the energy range of 230 keV-22 MeV, produced via 7Li(n,p) 7Be, 2H(d,n) 3He and 3H(d,n) 4He reactions in a Tandem Van de Graff accelerator. The gamma ray contribution to the obtained pulse height distribution and the resolution of the counters as a function of shaping time constant and applied high voltage were studied.

  2. Surface Waves on the Superfluids ^3He and ^4He

    NASA Astrophysics Data System (ADS)

    Manninen, M. S.; Ranni, A.; Rysti, J.; Todoshchenko, I. A.; Tuoriniemi, J. T.

    2016-06-01

    Free surface waves were examined both in superfluids ^3He and ^4He with the premise that these inviscid media would represent ideal realizations for this fluid dynamics problem. The work in ^3He is one of the first of its kind, but in ^4He, it was possible to produce a much more complete set of data for meaningful comparison with theoretical models. Most measurements were performed at the zero temperature limit, meaning T< 100 mK for ^4He and T˜ 100 μ K for ^3He. Dozens of surface wave resonances, including up to 11 overtones, were observed and monitored as the liquid depth in the cell was varied. Despite of the wealth of data, perfect agreement with the constructed theoretical models could not be achieved.

  3. Superfluidity of Dense {sup 4}He in Vycor

    SciTech Connect

    Khairallah, Saad A.; Ceperley, D.M.

    2005-10-28

    We calculate properties of a model of {sup 4}He in Vycor using the path integral Monte Carlo method. We find that {sup 4}He forms a distinct layered structure with a highly localized first layer, a disordered second layer with some atoms delocalized and able to give rise to the observed superfluid response, and higher layers of nearly perfect crystals. The addition of a single {sup 3}He atom was enough to bring down the total superfluidity by blocking the exchange in the second layer. Our results are consistent with the persistent liquid-layer model to explain the observations. Such a model may be relevant to the experiments on bulk solid {sup 4}He, if there is a fine network of grain boundaries in those systems.

  4. Heat Capacity of Dilute 3He-4He Monolayer Films

    NASA Astrophysics Data System (ADS)

    Morishita, Masashi

    2016-05-01

    The heat capacities of a small amount of 3He dissolved in monolayer 4He films are measured to clarify natures of monolayer 4He films. With increasing areal density, the measured heat capacities gradually increase and subsequently gradually decrease. With further increase in areal density, the measured heat capacity rapidly decreases to zero over a very narrow areal density range near that of the sqrt{3} × sqrt{3} phase. These slightly complex areal-density variations and dependence on 3He concentration are discussed from the viewpoint of the known properties of 4He films. The behaviors can be explained. However, the expected two-dimensional gas-liquid or gas-solid coexistence is not observed in this study.

  5. Evidence for a superglass state in solid 4He.

    PubMed

    Hunt, B; Pratt, E; Gadagkar, V; Yamashita, M; Balatsky, A V; Davis, J C

    2009-05-01

    Although solid helium-4 (4He) may be a supersolid, it also exhibits many phenomena unexpected in that context. We studied relaxation dynamics in the resonance frequency f(T) and dissipation D(T) of a torsional oscillator containing solid 4He. With the appearance of the "supersolid" state, the relaxation times within f(T) and D(T) began to increase rapidly together. More importantly, the relaxation processes in both D(T) and a component of f(T) exhibited a complex synchronized ultraslow evolution toward equilibrium. Analysis using a generalized rotational susceptibility revealed that, while exhibiting these apparently glassy dynamics, the phenomena were quantitatively inconsistent with a simple excitation freeze-out transition because the variation in f was far too large. One possibility is that amorphous solid 4He represents a new form of supersolid in which dynamical excitations within the solid control the superfluid phase stiffness.

  6. Dendritic crystal growth in pure /sup 4/He

    SciTech Connect

    Franck, J.P.; Jung, J.

    1986-08-01

    Dendritic crystal growth of pure hcp and fcc /sup 4/He was observed at pressures between 210 and 6500 bar. Dendrite morphology depends on fluid supercooling and crystal phase. At large supercooling, dendrites with side arms are observed, whereas at low supercooling dendrites grow without side arms. The morpholpogy of hcp /sup 4/He dendrites is strongly influenced by crystalline anisotropy. Comparison with present theories of dendrite growth show good agreement with the power law dependencies of velocity, tip radius, and Peclet number on supercooling. Numerically, theory predicts much larger velocities than are observed. The stability parameter sigma is found to be much smaller than theoretically predicted.

  7. Response of a Mechanical Oscillator in Solid 4He

    NASA Astrophysics Data System (ADS)

    Ahlstrom, S. L.; Bradley, D. I.; Človečko, M.; Fisher, S. N.; Guénault, A. M.; Guise, E. A.; Haley, R. P.; Kolosov, O.; Kumar, M.; McClintock, P. V. E.; Pickett, G. R.; Polturak, E.; Poole, M.; Todoshchenko, I.; Tsepelin, V.; Woods, A. J.

    2014-04-01

    We present the first measurements of the response of a mechanical oscillator in solid 4He. We use a lithium niobate tuning fork operating in its fundamental resonance mode at a frequency of around 30 kHz. Measurements in solid 4He were performed close to the melting pressure. The tuning fork resonance shows substantial frequency shifts on cooling from around 1.5 K to below 10 mK. The response shows an abrupt change at the bcc-hcp transition. At low temperatures, below around 100 mK, the resonance splits into several overlapping resonances.

  8. Photodisintegration of $^4$He into p+t

    SciTech Connect

    R. Nasseripour, B.L. Berman, N. Benmouna, Y. Ilieva, J.-M. Laget

    2009-10-01

    The two-body photodisintegration of $^4$He into a proton and a triton has been studied using the CEBAF Large-Acceptance Spectrometer (CLAS) at Jefferson Laboratory. Real photons produced with the Hall-B bremsstrahlung-tagging system in the energy range from 0.35 to 1.55 GeV were incident on a liquid $^4$He target. This is the first measurement of the photodisintegration of $^4$He above 0.4 GeV. The differential cross sections for the $\\gamma$$^4$He$\\to pt$ reaction have been measured as a function of photon-beam energy and proton-scattering angle, and are compared with the latest model calculations by J.-M. Laget. At 0.6-1.2 GeV, our data are in good agreement only with the calculations that include three-body mechanisms, thus confirming their importance. These results reinforce the conclusion of our previous study of the three-body breakup of $^3$He that demonstrated the great importance of three-body mechanisms in the energy region 0.5-0.8 GeV .

  9. Nuclear polarization corrections to the μ4He+ Lamb shift.

    PubMed

    Ji, C; Nevo Dinur, N; Bacca, S; Barnea, N

    2013-10-01

    Stimulated by the proton radius conundrum, measurements of the Lamb shift in various light muonic atoms are planned at PSI. The aim is to extract the rms charge radius with high precision, limited by the uncertainty in the nuclear polarization corrections. We present an ab initio calculation of the nuclear polarization for μ(4)He(+) leading to an energy correction in the 2S-2P transitions of δ(pol)(A)=-2.47 meV ±6%. We use two different state-of-the-art nuclear Hamiltonians and utilize the Lorentz integral transform with hyperspherical harmonics expansion as few-body methods. We take into account the leading multipole contributions, plus Coulomb, relativistic, and finite-nucleon-size corrections. Our main source of uncertainty is the nuclear Hamiltonian, which currently limits the attainable accuracy. Our predictions considerably reduce the uncertainty with respect to previous estimates and should be instrumental to the μ(4)He(+) experiment planned for 2013.

  10. Sodium dimers on the surface of liquid {sup 4}He

    SciTech Connect

    Ancilotto, F.; DeToffol, G.; Toigo, F.

    1995-12-01

    We have studied the structure of a sodium dimer interacting with liquid {sup 4}He. We calculated the equilibrium configuration and binding energy of a Na{sub 2} molecule solvated in a bulk liquid {sup 4}He ``bubble`` and near the liquid-vapor interface ``dimple`` by using a density-functional approach. We find that the solvated molecule is a metastable state, while the the lowest energy bound state occurs when the molecule lies flat on the surface of the liquid. The binding energy for the ``erect`` dimer is only {similar_to}1 K higher than the flat dimer, with no potential energy barrier between the two orientations, implying relatively free rotations of the molecule on the surface. The small effects of the liquid environment on the vibrational properties of the dimer are investigated.

  11. Overview on Solid 4He and the Issue of Supersolidity

    NASA Astrophysics Data System (ADS)

    Chan, M. H. W.; Hallock, R. B.; Reatto, L.

    2013-09-01

    Here we provide an overview of the status of the field of solid 4He with a focus on the recent theoretical and experimental activities stimulated by the 2004 experiments of Kim and Chan. The overview attempts to place the experimental and theoretical work in context, to respect the historical flow of the field and discuss our present understanding of the question of supersolidity in 4He. The possibility of supersolidity in cold atoms and in other systems is also addressed. Special issues of the Journal of Low Temperature Physics (168(3/4), 2012; 169(3/4), 2012), in addition to this issue, have been devoted to this subject and this overview is meant to accompany those issues of the journal.

  12. Bose-Einstein condensation in liquid 4He under pressure

    SciTech Connect

    Glyde, Henry R; Omar Diallo, Souleymane; Azuah, Richard T; Kirichek, Oleg; Taylor, Jon W.

    2011-01-01

    We present neutron scattering measurements of Bose-Einstein condensation, the atomic momen- tum distribution and Final State effects in liquid 4He under pressure. The condensate fraction at low temperature is found to decrease from n0 = 7.25 0.75% at SVP (p 0) to n0 = 3.2 0.75% at pressure p = 24 bar. This indicates an n0 = 3.0% in the liquid at the liquid/solid co-existence line (p = 25.3 bar). The atomic momentum distribution n(k) has high occupation of low k states and differs significantly from a Gaussian (e.g. a classical n(k)). Both n(k) and the Final state function broaden with increasing pressure, reflecting the increased localization of the 4He in space under increased pressure.

  13. NOVEL CONCEPTS FOR ISOTOPIC SEPARATION OF 3HE/4HE

    SciTech Connect

    Roy, L.; Nigg, H.; Watson, H.

    2012-09-04

    The research outlined below established theoretical proof-of-concept using ab initio calculations that {sup 3}He can be separated from {sup 4}He by taking advantage of weak van der Waals interactions with other higher molecular weight rare gases such as xenon. To the best of our knowledge, this is the only suggested method that exploits the physical differences of the isotopes using a chemical interaction.

  14. Cross-checking groundwater age by 4He and 14C dating in a granite, Tono area, central Japan

    NASA Astrophysics Data System (ADS)

    Hasegawa, Takuma; Nakata, Kotaro; Tomioka, Yuichi; Goto, Kazuyuki; Kashiwaya, Koki; Hama, Katsuhiro; Iwatsuki, Teruki; Kunimaru, Takanori; Takeda, Masaki

    2016-11-01

    Groundwater dating was performed simultaneously by the 4He and 14C methods in granite of the Tono area in central Japan. Groundwater was sampled at 30 packed-off sections of six 1000-m boreholes. 4He concentrations increased and 14C concentrations decreased along a groundwater flow path on a topographic gradient. 4He ages were calculated by using the in situ 4He production rate derived from the porosity, density, and U and Th content of the rock, neglecting external flux. 14C ages were calculated with a noncorrected model in which the initial 14C content was 100 percent of the modern radiocarbon level (Co = 100 pmC), a statistical model using the average 14C content of tritium-bearing samples (Co = 46.4 pmC), and a δ13C model based on the isotopic mass balance. Although the absolute 14C ages calculated by the models were different, the relative 14C ages were almost identical. The relative 14C ages were considered reliable because dissolved inorganic carbon has no significant geochemical reactions in granite. The relation between the 4He ages and the noncorrected 14C ages was [4He age] = 1.15 [14C age] + 7200 (R2 = 0.81), except in the discharge area. The slope of this relation was equivalent to unity, which indicates that the 4He accumulation rate is confirmed by the relative 14C ages. Moreover, the accumulated 3He/4He ratio was equivalent to that derived from the 6Li(α,n)3H reaction in granite. These results show that the accumulated He is of crustal origin, produced in situ without external flux, except in the discharge area. The intercept value of 7200 a implies that the 14C concentrations were diluted due to geochemical reactions. Tritium-bearing samples supported this result. Simultaneous measurements make it feasible to estimate the accumulation rate of 4He and initial dilution of 14C, which cannot be done with a single method. Cross-checking groundwater dating has the potential to provide more reliable groundwater ages. The circulation time of the

  15. Hyperspherical coupled channel calculations of energy and structure of 4He-4He-Li+ and its isotopic combinations

    NASA Astrophysics Data System (ADS)

    Liu, Min-min; Wu, Meng-Shan; Han, Hui-li; Shi, Ting-yun

    2016-07-01

    The ground state vibrational energy and spatial features of 4He-4He-Li+ and its triatomic isotopic complexes are studied using the slow variable discretization (SVD) method in the hyperspherical coordinates for the zero total angular momentum. Our results show that the dominant structure of the system is an isosceles triangle with the shorter side associated with the two Li+-He distances using the sum-of-potential approximation. Corrections caused by the induced dipole-induced dipole interactions on the He atoms are also investigated. The effects are seen to be small and have a minor influence on the binding energy and the structure of present system. The results are also compared with the full ab initio calculations including all the three-body interactions and information of three-body corrections is obtained.

  16. Hyperspherical coupled channel calculations of energy and structure of (4)He-(4)He-Li(+) and its isotopic combinations.

    PubMed

    Liu, Min-Min; Wu, Meng-Shan; Han, Hui-Li; Shi, Ting-Yun

    2016-07-21

    The ground state vibrational energy and spatial features of (4)He-(4)He-Li(+) and its triatomic isotopic complexes are studied using the slow variable discretization (SVD) method in the hyperspherical coordinates for the zero total angular momentum. Our results show that the dominant structure of the system is an isosceles triangle with the shorter side associated with the two Li(+)-He distances using the sum-of-potential approximation. Corrections caused by the induced dipole-induced dipole interactions on the He atoms are also investigated. The effects are seen to be small and have a minor influence on the binding energy and the structure of present system. The results are also compared with the full ab initio calculations including all the three-body interactions and information of three-body corrections is obtained. PMID:27448884

  17. Solidification of 4He clusters adsorbed on graphene

    NASA Astrophysics Data System (ADS)

    Markić, L. Vranješ; Stipanović, P.; Bešlić, I.; Zillich, R. E.

    2016-07-01

    We determined the ground state of He4N clusters adsorbed on one side of graphene for selected cluster sizes in the range from N =20 to N =127 . For all investigated clusters variational and diffusion Monte Carlo simulations were performed at T =0 K, and in addition for a selected subset finite temperature path integral Monte Carlo. At T =0 K the liquid or solid character of each cluster was investigated by restricting the phase using corresponding importance sampling trial-wave functions. The 4He-graphene interaction was modeled as a sum of individual 4He-C interactions, where both isotropic and anisotropic models were tested; also the effect of the substrate-mediated McLachlan interaction was investigated. We have found homogeneous crystallization in models of anisotropic interactions, starting from clusters with N =26 atoms in simulations without the McLachlan interaction, and between N =37 and 61 when it is included. The atoms become increasingly delocalized as one moves from the center of the cluster to the perimeter, evidenced by the Lindemann parameter. On the other hand, in the case of the isotropic interaction model, a liquidlike structure is more favorable for all considered cluster sizes. We use a liquid-drop model to extrapolate the energy per particle to the N →∞ limit, and the results are compared with the values obtained in studies of bulk 4He on graphene. Low-temperature path integral Monte Carlo simulations are in agreement with ground-state results.

  18. Density pattern in supercritical flow of liquid {sup 4}He

    SciTech Connect

    Ancilotto, F.; Toigo, F.; Dalfovo, F.; Pitaevskii, L.P.

    2005-03-01

    A density-functional theory is used to investigate the instability arising in superfluid {sup 4}He as it flows at velocity u just above the Landau critical velocity of rotons v{sub c}. Confirming an early theoretical prediction by one of us [JETP Lett. 39, 511 (1984)], we find that a stationary periodic modulation of the density occurs, with amplitude proportional to (u-v{sub c}){sup 1/2} and wave vector equal to the roton wave vector. This density pattern is studied for supercritical flow both in bulk helium and in a channel of nanometer cross section.

  19. Quantum Monte Carlo Simulation of Overpressurized Liquid {sup 4}He

    SciTech Connect

    Vranjes, L.; Boronat, J.; Casulleras, J.; Cazorla, C.

    2005-09-30

    A diffusion Monte Carlo simulation of superfluid {sup 4}He at zero temperature and pressures up to 275 bar is presented. Increasing the pressure beyond freezing ({approx}25 bar), the liquid enters the overpressurized phase in a metastable state. In this regime, we report results of the equation of state and the pressure dependence of the static structure factor, the condensate fraction, and the excited-state energy corresponding to the roton. Along this large pressure range, both the condensate fraction and the roton energy decrease but do not become zero. The roton energies obtained are compared with recent experimental data in the overpressurized regime.

  20. Classical Rotational Inertia of Solid {sup 4}He

    SciTech Connect

    Dash, J.G.; Wettlaufer, J.S.

    2005-06-17

    The observation of reduced rotational inertia in a cell containing solid {sup 4}He has been interpreted as evidence for superfluidity of the solid. We propose an alternative explanation: slippage of the solid, due to grain boundary premelting between the solid and dense adsorbed layers at the container wall. We calculate the range of film thickness, and determine the viscosity that will account for the missing rotational inertia. Grain boundary premelting also explains inertial anomalies in an earlier study of solid helium in porous glass and indicates that the liquid is partially superfluid.

  1. Electron-Induced Neutron Knockout from 4He

    NASA Astrophysics Data System (ADS)

    Misiejuk, A.; Papandreou, Z.; Voutier, E.; Bauer, Th. S.; Blok, H. P.; Boersma, D. J.; den Bok, H. W.; Bruins, E. E.; Farzanpay, F.; Grüner, K.; Hesselink, W. H.; Huber, G. M.; Jans, E.; Kalantar-Nayestanaki, N.; Kasdorp, W.-J.; Konijn, J.; Laget, J.-M.; Lapikás, L.; Lolos, G. J.; Onderwater, G. J.; Pellegrino, A.; Schroevers, R.; Spaltro, C. M.; Starink, R.; van der Steenhoven, G.; Steiger, J. J.; Visschers, J. L.; Willering, H. W.; Yeomans, D. M.

    2002-10-01

    The differential cross section for electron-induced neutron knockout in the reaction 4He(e,e'n)3He has been measured for the first time with a statistical accuracy of 11%. The experiment was performed in quasielastic kinematics at a momentum transfer of 300 MeV/c and in the missing-momentum range of 25-70 MeV/c. The comparison of the data with theoretical calculations shows an impressive increase of the cross section resulting from final state interaction effects. Specifically , the p-n charge-exchange process dominates the cross section in this kinematical regime.

  2. Compression-Driven Mass Flow in Bulk Solid 4He

    NASA Astrophysics Data System (ADS)

    Cheng, Zhi Gang; Beamish, John

    2016-07-01

    Mass flow has been observed in solid 4He coexisting with superfluid confined in Vycor, but its physical mechanism remains an open question. Here we report observations of flow in experiments in which Vycor has been eliminated, allowing us to study the intrinsic flow in solid 4He without the complications introduced by the presence of superfluid and the associated solid-liquid interfaces. By growing crystals with 3He concentration as low as x3=5 ×10-12, we also avoided the low temperature flow suppression observed in previous experiments and found that the flow rate continued to increase down to at least 28 mK without saturation. In addition, 3He concentrations of 120 ppb, which suppressed most of the low temperature flow in previous experiments, had no effect in our samples. The larger 3He concentrations needed to block the bulk solid flow suggest that the mass flow involves a larger area, such as disordered liquid layer on solid surface and grain boundaries.

  3. Sliding Wigner solid on liquid {sup 4}He

    SciTech Connect

    Shirahama, Keiya; Kono, Kimitoshi

    1996-08-01

    The authors report a systematic experimental study of the anomalous nonlinear magnetotransport in the Wigner solid (WS) trapped on a liquid {sup 4}He surface. The ac Corbino conductivity {sigma}{sub xx} exhibits an abrupt jump at a certain driving voltage. The threshold input voltage V{sub th} for the {sigma}{sub xx} jump varies as V{sub th} {proportional_to}B{sup {minus}0.8}{omega}{sup {minus}1}n{sub s}{sup 1.5}E{sub {perpendicular}}, where B, {omega}, n{sub s}, and E{sub {perpendicular}} are magnetic field, frequency, electron density and pressing electric field, respectively. The authors interpret the {sigma}{sub xx} jump as the transition between the WS accompanied with the periodic {sup 4}He surface deformation and the WS which decouples from the surface, due to the large driving force. A simple model is presented: The rigid-potential sliding model qualitatively explains the above mentioned behaviors of V{sub th}. They have found that the dependences of {sigma}{sub xx} on B and E{sub {perpendicular}} are different from those of the liquid phase. The anomalous behaviors of {sigma}{sub xx} play a crucial role on the sliding model.

  4. Compression-Driven Mass Flow in Bulk Solid ^{4}He.

    PubMed

    Cheng, Zhi Gang; Beamish, John

    2016-07-01

    Mass flow has been observed in solid ^{4}He coexisting with superfluid confined in Vycor, but its physical mechanism remains an open question. Here we report observations of flow in experiments in which Vycor has been eliminated, allowing us to study the intrinsic flow in solid ^{4}He without the complications introduced by the presence of superfluid and the associated solid-liquid interfaces. By growing crystals with ^{3}He concentration as low as x_{3}=5×10^{-12}, we also avoided the low temperature flow suppression observed in previous experiments and found that the flow rate continued to increase down to at least 28 mK without saturation. In addition, ^{3}He concentrations of 120 ppb, which suppressed most of the low temperature flow in previous experiments, had no effect in our samples. The larger ^{3}He concentrations needed to block the bulk solid flow suggest that the mass flow involves a larger area, such as disordered liquid layer on solid surface and grain boundaries. PMID:27447513

  5. Ab initio many-body calculations of nucleon-4He scattering with three-nucleon forces

    DOE PAGES

    Hupin, Guillaume; Langhammer, Joachim; Navratil, Petr; Quaglioni, Sofia; Calci, Angelo; Roth, Robert

    2013-11-27

    We extend the ab initio no-core shell model/resonating-group method to include three-nucleon (3N) interactions for the description of nucleon-nucleus collisions. We outline the formalism, give algebraic expressions for the 3N-force integration kernels, and discuss computational aspects of two alternative implementations. The extended theoretical framework is then applied to nucleon-4He elastic scattering using similarity-renormalization-group (SRG)-evolved nucleon-nucleon plus 3N potentials derived from chiral effective field theory. We analyze the convergence properties of the calculated phase shifts and explore their dependence upon the SRG evolution parameter. We include up to six excited states of the 4He target and find significant effects from themore » inclusion of the chiral 3N force, e.g., it enhances the spin-orbit splitting between the 3/2– and 1/2– resonances and leads to an improved agreement with the phase shifts obtained from an accurate R-matrix analysis of the five-nucleon experimental data. As a result, we find remarkably good agreement with measured differential cross sections at various energies below the d+3H threshold, while analyzing powers manifest larger deviations from experiment for certain energies and angles.« less

  6. Quantized Vortex State in hcp Solid 4He

    NASA Astrophysics Data System (ADS)

    Kubota, Minoru

    2012-11-01

    The quantized vortex state appearing in the recently discovered new states in hcp 4He since their discovery (Kim and Chan, Nature, 427:225-227, 2004; Science, 305:1941, 2004) is discussed. Special attention is given to evidence for the vortex state as the vortex fluid (VF) state (Anderson, Nat. Phys., 3:160-162, 2007; Phys. Rev. Lett., 100:215301, 2008; Penzev et al., Phys. Rev. Lett., 101:065301, 2008; Nemirovskii et al., arXiv:0907.0330, 2009) and its transition into the supersolid (SS) state (Shimizu et al., arXiv:0903.1326, 2009; Kubota et al., J. Low Temp. Phys., 158:572-577, 2010; J. Low Temp. Phys., 162:483-491, 2011). Its features are described. The historical explanations (Reatto and Chester, Phys. Rev., 155(1):88-100, 1967; Chester, Phys. Rev. A, 2(1):256-258, 1970; Andreev and Lifshitz, JETP Lett., 29:1107-1113, 1969; Leggett, Phys. Rev. Lett., 25(22), 1543-1546, 1970; Matsuda and Tsuneto, Prog. Theor. Phys., 46:411-436, 1970) for the SS state in quantum solids such as solid 4He were based on the idea of Bose Einstein Condensation (BEC) of the imperfections such as vacancies, interstitials and other possible excitations in the quantum solids which are expected because of the large zero-point motions. The SS state was proposed as a new state of matter in which real space ordering of the lattice structure of the solid coexists with the momentum space ordering of superfluidity. A new type of superconductors, since the discovery of the cuprate high T c superconductors, HTSCs (Bednorz and Mueller, Z. Phys., 64:189, 1986), has been shown to share a feature with the vortex state, involving the VF and vortex solid states. The high T c s of these materials are being discussed in connection to the large fluctuations associated with some other phase transitions like the antiferromagnetic transition in addition to that of the low dimensionality. The supersolidity in the hcp solid 4He, in contrast to the new superconductors which have multiple degrees of freedom of

  7. Dissipation of Quasiclassical Turbulence in Superfluid ^{4}He.

    PubMed

    Zmeev, D E; Walmsley, P M; Golov, A I; McClintock, P V E; Fisher, S N; Vinen, W F

    2015-10-01

    We compare the decay of turbulence in superfluid ^{4}He produced by a moving grid to the decay of turbulence created by either impulsive spin-down to rest or by intense ion injection. In all cases, the vortex line density L decays at late time t as L∝t^{-3/2}. At temperatures above 0.8 K, all methods result in the same rate of decay. Below 0.8 K, the spin-down turbulence maintains initial rotation and decays slower than grid turbulence and ion-jet turbulence. This may be due to a decoupling of the large-scale superfluid flow from the normal component at low temperatures, which changes its effective boundary condition from no-slip to slip.

  8. Dislocation Structure and Mobility in hcp ^{4}He.

    PubMed

    Landinez Borda, Edgar Josué; Cai, Wei; de Koning, Maurice

    2016-07-22

    Using path-integral Monte Carlo simulations, we assess the core structure and mobility of the screw and edge basal-plane dislocations in hcp ^{4}He. Our findings provide key insights into recent interpretations of giant plasticity and mass flow junction experiments. First, both dislocations are dissociated into nonsuperfluid Shockley partial dislocations separated by ribbons of stacking fault, suggesting that they are unlikely to act as one-dimensional channels that may display Lüttinger-liquid-like behavior. Second, the centroid positions of the partial cores are found to fluctuate substantially, even in the absence of applied shear stresses. This implies that the lattice resistance to motion of the partial dislocations is negligible, consistent with the recent experimental observations of giant plasticity. Further results indicate that both the structure of the partial cores and the zero-point fluctuations play a role in this extreme mobility. PMID:27494477

  9. X-rays from antiprotonic3He and4He

    NASA Astrophysics Data System (ADS)

    Schneider, M.; Bacher, R.; Blüm, P.; Gotta, D.; Heitlinger, K.; Kunold, W.; Rohmann, D.; Egger, J.; Simons, L. M.; Elsener, K.

    1991-06-01

    Antiprotonic X-rays from the helium isotopes have been observed at pressures of 36, 72, 375 and 600 mbar. The antiproton beam from LEAR with momenta of 309 and 202 MeV/c has been stopped at these pressures using the cyclotron trap. The X-rays were detected with Si (Li) and intrinsic Ge semiconductor detectors. Absolute X-ray yields were determined and the strong-interaction 2p shifts and the 2p and 3d broadenings measured to be ɛ2p=(-17±4) eV, Γ2p=(25±9) eV and Γ3d=(2.14 ±0.18) meV for ¯p3He and ɛ2p=(-18±2) eV, Γ2p =(45±5) eV and Γ3d=(2.36±0.10) meV for ¯p4He.

  10. Dislocation Structure and Mobility in hcp 4He

    NASA Astrophysics Data System (ADS)

    Landinez Borda, Edgar Josué; Cai, Wei; de Koning, Maurice

    2016-07-01

    Using path-integral Monte Carlo simulations, we assess the core structure and mobility of the screw and edge basal-plane dislocations in hcp 4He. Our findings provide key insights into recent interpretations of giant plasticity and mass flow junction experiments. First, both dislocations are dissociated into nonsuperfluid Shockley partial dislocations separated by ribbons of stacking fault, suggesting that they are unlikely to act as one-dimensional channels that may display Lüttinger-liquid-like behavior. Second, the centroid positions of the partial cores are found to fluctuate substantially, even in the absence of applied shear stresses. This implies that the lattice resistance to motion of the partial dislocations is negligible, consistent with the recent experimental observations of giant plasticity. Further results indicate that both the structure of the partial cores and the zero-point fluctuations play a role in this extreme mobility.

  11. Theoretical modeling of electron mobility in superfluid 4He

    NASA Astrophysics Data System (ADS)

    Aitken, Frédéric; Bonifaci, Nelly; von Haeften, Klaus; Eloranta, Jussi

    2016-07-01

    The Orsay-Trento bosonic density functional theory model is extended to include dissipation due to the viscous response of superfluid 4He present at finite temperatures. The viscous functional is derived from the Navier-Stokes equation by using the Madelung transformation and includes the contribution of interfacial viscous response present at the gas-liquid boundaries. This contribution was obtained by calibrating the model against the experimentally determined electron mobilities from 1.2 K to 2.1 K along the saturated vapor pressure line, where the viscous response is dominated by thermal rotons. The temperature dependence of ion mobility was calculated for several different solvation cavity sizes and the data are rationalized in the context of roton scattering and Stokes limited mobility models. Results are compared to the experimentally observed "exotic ion" data, which provides estimates for the corresponding bubble sizes in the liquid. Possible sources of such ions are briefly discussed.

  12. Dynamics of Laser Ablation in Superfluid ^4He

    NASA Astrophysics Data System (ADS)

    Buelna, X.; Popov, E.; Eloranta, J.

    2016-10-01

    Pulsed laser ablation of metal targets immersed in superfluid ^4He is visualized by time-resolved shadowgraph photography and the products are analyzed by post-experiment atomic force microscopy (AFM) measurements. The expansion dynamics of the gaseous ablation half-bubble on the target surface appears underdamped and follows the predicted behavior for the thermally induced bubble growth mechanism. An inherent instability of the ablation bubble appears near its maximum radius and no tightly focused cavity collapse or rebound events are observed. During the ablation bubble retreat phase, the presence of sharp edges in the target introduces flow patterns that lead to the creation of large classical vortex rings. Furthermore, on the nanometer scale, AFM data reveal that the metal nanoparticles created by laser ablation are trapped in spherical vortex tangles and quantized vortex rings present in the non-equilibrium liquid.

  13. cap alpha. /sup 4/He elastic scattering at high energies

    SciTech Connect

    Usmani, A.A.; Ahmad, I.; Usmani, Q.N.

    1989-03-01

    Differential cross sections for ..cap alpha.. /sup 4/He elastic scattering have been calculated at incident ..cap alpha..-particle momenta of 4.32, 5.07, and 7.0 GeV/c within the framework of Glauber multiple scattering theory. The full Glauber amplitude has been calculated using the Monte Carlo method for evaluating multidimensional integrals. We found that, in general, the more realistic double-Gaussian model for the density brings theory closer to experiment as compared to the generally used single-Gaussian model in some momentum transfer regions. Our results with the double-Gaussian model and an acceptable set of NN parameters are in fairly good agreement with the experimental data at 4.32 and 5.07 GeV/c.

  14. Theoretical modeling of electron mobility in superfluid (4)He.

    PubMed

    Aitken, Frédéric; Bonifaci, Nelly; von Haeften, Klaus; Eloranta, Jussi

    2016-07-28

    The Orsay-Trento bosonic density functional theory model is extended to include dissipation due to the viscous response of superfluid (4)He present at finite temperatures. The viscous functional is derived from the Navier-Stokes equation by using the Madelung transformation and includes the contribution of interfacial viscous response present at the gas-liquid boundaries. This contribution was obtained by calibrating the model against the experimentally determined electron mobilities from 1.2 K to 2.1 K along the saturated vapor pressure line, where the viscous response is dominated by thermal rotons. The temperature dependence of ion mobility was calculated for several different solvation cavity sizes and the data are rationalized in the context of roton scattering and Stokes limited mobility models. Results are compared to the experimentally observed "exotic ion" data, which provides estimates for the corresponding bubble sizes in the liquid. Possible sources of such ions are briefly discussed. PMID:27475346

  15. Σ production from targets of ^4He and ^13C

    NASA Astrophysics Data System (ADS)

    Chrien, R. E.

    1996-10-01

    One of the abiding issues in hypernuclear research has been the question of the formation of nuclear bound states incorporating the Σ-hyperon. The recent increases in beam intensity at the Brookhaven AGS have enabled us to obtain a high statistics study on the production of Σ-hyperons on a ^4He target. Earlier research using stopped kaons at KEK indicated the presence of structure in the (K^-,π^-) reaction, and led to the postulate of a Σ bound state. That structure has now been definitely confirmed in the in-flight kaon experiment at the LESB2 beam line and Moby-Dick spectrometer. An improved measurement of the binding energy of the presumed state will be reported, together with a production cross section. In addition, both (K^-,π^-) and (K^-,π^+) reactions on ^13C have been studied and will be compared to similar measurements on ^9Be.

  16. Observation of melting of solid 4He by sound wave

    NASA Astrophysics Data System (ADS)

    Okuda, Y.; Yamazaki, S.; Yoshida, T.; Fujii, H.; Matsumoto, K.

    1999-03-01

    We have observed the crystal melting, or the depletion of the solid/liquid interface where the strong pulsed sound beam was passing. The crystal was produced around 0.8 K with the atomically rough horizontal surface sitting in the middle of the sample cell. The interface was very mobile which was confirmed by an easy excitation of the crystallization/melting wave. When the received signal through the interface was monitored as a function of the input power, a sudden saturation of the received signal was observed at some power. For well above that power, the melting of the interface was visible through a video camera for both the cases of the sound emission from fluid-side and solid-side. This would be the first observation of sound induced melting of solid 4He.

  17. Magnetic-field-assisted atomic polarization spectroscopy of 4 He

    NASA Astrophysics Data System (ADS)

    Li, Sheng; Wang, Haidong; Wu, Teng; Peng, Xiang; Guo, Hong; Cream Team

    2016-05-01

    Atomic polarization spectroscopy (PS) is a high resolution sub-Doppler atomic spectroscopic technique with free modulation. It is always desirable to obtain a PS signal with zero background as it can provide a more preferable laser frequency stabilization performance. There are many factors that can affect the PS signal background, i.e., the laser power, the laser polarization and the magnetic field. Here, we demonstrate a method for observing and analyzing the effects on the PS signal of 4 He under different magnetic fields. At the beginning, under nearly zero magnetic field, the large asymmetrical PS signal background has been observed and cannot be eliminated by only optically adjusting. Then, we find that the PS signal profile can be changed and controlled by varying the magnetic field with transverse or longitudinal direction and different intensity. The optimized PS signal with symmetrical dispersive profile and zero background is obtained when the magnetic field is chosen and controlled in the transverse direction and more than 20000nT intensity. Similar phenomenon cannot be observed under the longitudinal magnetic field. A theoretical model is also presented, which explains and agrees well with our experimental results.

  18. Correlation of Excess Enthalpy and ^4He Production: a Review

    NASA Astrophysics Data System (ADS)

    Miles, M. H.

    2004-03-01

    Three different sets of experiments conducted in the Navy Laboratory (NAWCWD) at China Lake, California (1990-1994) clearly established that helium-4 is the main fusion product in the Pd/D_2O+LiOD electrolysis system(P.A. Mosier-Boss, S.R. Chubb, M. Fleischmann, M. Imam, M. H. Miles, S. Szpak, TR 1862, SPAWAR Systems Center, San Diego; see http://www.lenr-canr.org/acrobat/MosierBossthermaland.pdf). A correlation between excess enthalpy and excess helium-4 was measured in 18 out of 21 experiments. The observation of no excess enthalpy was correlated with no excess helium in 12 out of 12 experiments. Thus 30 out of 33 experiments agree with the hypothesis that the excess enthalpy produced in cold fusion studies is correlated with helium-4 production: d+darrow ^4He + 23.8 MeV. Furthermore, the measured rate of helium-4 production was always in the appropriate range of 10^1^0 to 10^1^2 atoms per second per watt of excess power.

  19. Creep in solid 4He at temperatures below 1 K

    NASA Astrophysics Data System (ADS)

    Zhuchkov, V. A.; Lisunov, A. A.; Maidanov, V. A.; Neoneta, A. S.; Rubanskyi, V. Yu.; Rubets, S. P.; Rudavskii, E. Ya.; Smirnov, S. N.

    2015-03-01

    Creep in solid 4He at temperatures of ˜100-1000 mK is studied experimentally by detecting the flow of helium through a frozen porous membrane under a constant external force. Creep curves are measured for different temperatures and mechanical stresses. This method has made it possible to detect low creep rates in helium down to the lowest temperatures in these experiments. It is found that throughout this temperature range, creep is thermally activated and the activation energy decreases with falling temperature and increasing mechanical stress. An analysis shows that for temperatures above ≈500 mK, Nabarro-Herring diffusive creep takes place in solid helium with mass transfer by self diffusion of atoms and a counterflow of vacancies. The experimental data have been used to obtain the self-diffusion coefficient as a function of temperature for different stresses. At temperatures below ≈500 mK creep takes place at a very low flow rate (˜10-13 cm/s) and a very low activation energy (˜0.5-0.7 K), while the creep mechanism remains unclear.

  20. Stress induced roughening of superclimbing dislocation in solid 4He

    NASA Astrophysics Data System (ADS)

    Aleinikava, Darya; Kuklov, Anatoly

    2011-03-01

    We investigate numerically superclimb of dislocation in solid 4 He biased by externally imposed chemical potential μ . The effective action takes into account quantum phase slips in the core superfluid as well as the core displacement in Peierls potential within the Granato-Lücke string model. The bias produces stress on the core and this can result in dislocation roughening. Such roughening is characterized by hysteretic behavior at temperatures (T) below some threshold Thyst . At T >Thyst strongresonantpeaksdevelopinthedislocationdifferentialresponse . Thesepeaksexhibitperiodicbehaviorvs μ, with the period determined by Peierls potential and dislocation length. We explain these effects by thermally assisted tunneling of jog-antijog pairs across the barrier created by Peierls potential and the bias. Since superclimbing is controlled by core superflow, speed of sound along the superfluid core exhibits dip-like features at the peak positions. We propose that this effect is seen in the mass transport experiment. We acknowledge support by NSF, grants PHY1005527 and PHY0653135,and by CUNY, grant 63071-00 41.

  1. Critical behavior of liquid {sup 4}He at negative pressures

    SciTech Connect

    Campbell, C.E.; Folk, R.; Krotscheck, E.

    1996-10-01

    The authors examine the equation of state of liquid {sup 4}He at negative pressures close to the spinodal density {rho}{sub s} where the hydrodynamic speed of sound vanishes. The non-analytic behavior of the equation of state and the speed of sound in the vicinity of the spinodal density are calculated in two and in three dimensions; they find for the speed of sound the non-analytic behavior mc{sub s}{sup 2} {approximately} ({rho}-{rho}{sub s}){sup 2/5} in three dimensions and mc{sub s}{sup 2} {approximately} [({rho}-{rho}{sub s})/{vert_bar}ln({rho}-{rho}{sub s}){vert_bar}]{sup 1/2} in two dimensions. The authors then examine the low density regime numerically, using a semianalytic microscopic theory. It is found that non-analytic exponents are visible only in a negligible density regime around the spinodal point. Estimates for the spinodal densities, and the range of critical fluctations are provided.

  2. 4He behavior in calcite filling viewed by (U-Th)/He dating, 4He diffusion and crystallographic studies

    NASA Astrophysics Data System (ADS)

    Cros, Alexandre; Gautheron, Cécile; Pagel, Maurice; Berthet, Patrick; Tassan-Got, Laurent; Douville, Eric; Pinna-Jamme, Rosella; Sarda, Philippe

    2014-01-01

    Fault-filling calcite crystals sampled from the Eocene/Oligocene Gondrecourt graben, Paris Basin, Eastern France, have been studied in order to test the potentiality of calcite (U-Th)/He dating, based on recognized He retention behavior in crystal lattice at surface temperature (Copeland et al., 2007). The samples have been selected because of their relatively old Eocene to Oligocene precipitation age and cold thermal history (<40 °C since precipitation). They were sorted into three main tectonic and morphological groups in order of precipitation, including (1) micro-fracture calcites, (2) breccia and associated geodic calcites, and (3) vein and associated geodic calcites. (U-Th)/He dating of 63 calcite fragments yields ages dispersed from 0.2 ± 0.02 to 35.8 ± 2.7 Ma, as well as two older dates of 117 ± 10 and 205 ± 28 Ma (1σ). These He ages correlate with grain chemistry, such as Sr, ΣREE concentrations or (La/Yb)N ratios, likely reflecting parent fluid evolution. Only the oldest He ages, which correspond to the most recently precipitated crystals, have preserved the total 4He budget since precipitation. To better understand both the age dispersion and why calcites precipitated earlier show younger ages, 4He diffusion experiments have been conducted on 10 Gondrecourt calcite fragments from 3 samples with He ages of ∼0.2-6 Ma. Additionally, a crystallographic investigation by X-ray diffraction (XRD) performed on similar samples reveals that crystal structure evolves with increasing temperature, beginning with micro-cracks and cleavage opening. These XRD results shed light on the (U-Th)/He data, indicating that, in fault-filling calcite, He retention is controlled by multiple diffusion domains (MDD) with various sizes, and therefore, evolves through time with strong consequences on (U-Th)/He age. We thus interpret the Gondrecourt calcite (U-Th)/He age scatter as a consequence of the production of defects due to successive calcite crystallization phases

  3. Thermal properties of {sup 4}He surfaces and interfaces

    SciTech Connect

    Clements, B.E.; Krotscheck, E. |; Tymczak, C.J.

    1997-05-01

    A first-principle quantum statistical mechanical theory is used to study the properties of thick liquid {sup 4}He films absorbed to the weakly binding substrates: Li, Na, and Cs. Values for the liquid-gas and solid-liquid surface energies are determined. By fitting, at long wavelengths, the film`s lowest energy mode with the standard expression for the ripplon energy, which depends on the liquid-gas surface energy, the authors obtain excellent agreement with the liquid-vacuum surface energy from recent experiments and also the one previously extracted from quantum liquid droplet calculations. The full spectrum of excitations for wave vectors less than 0.50 {Angstrom}{sup {minus}1} is calculated using a dynamical correlated basis function theory developed in earlier work, which includes multi-phonon scattering processes. Particle currents and transition densities are used to elucidate the nature of the excitations. At a coverage of 0.40 {Angstrom}{sup {minus}2}, the lowest mode shows no significant substrate dependence, and is recognized as being a ripplon propagating in the liquid film at the liquid-gas surface. A new effect is observed for the Cs substrate; the second lowest mode is qualitatively different than found on the other substrates and is identified as interfacial ripplon. In the other substrates the second mode is a volume mode altered somewhat by the high density inner liquid layers. The linewidths of these modes are also calculated. The dynamic excitations provide the input for the thermodynamic theory and the effects on the free energy, heat capacity, and thermal surface broadening of these films are studied as function of the nature of the excitations, the number of modes, and variations in the substrate potentials.

  4. Experiments on Rogue Waves in Superfluid 4He

    NASA Astrophysics Data System (ADS)

    Efimov, Viktor; McClintock, Peter; Ganshin, Andrei; Kolmakov, German; Mezhov-Deglin, Leonid

    2010-05-01

    We describe an experimental and theoretical study of nonlinear wave interactions in superfluid helium and report the observation of rogue waves. Rogue waves (or freak waves, or killer waves, or extreme waves) have long been recognized by sailors as a menace to shipping and are believed to have been responsible for the unexplained losses of vessels of all sizes, including e.g. 22 super-carriers between 1968 and 1994 [1, 2]. Rogue waves on the ocean are rare, and are much higher (and steeper) than all the other waves around them. They seem to appear from nowhere and subsequently to disappear without trace [3]. Following the famous 'New Year wave' measured by instruments on the Draupner North Sea oil rig at the beginning of 1995, the existence of oceanic rogue waves is no longer in doubt. There have been several suggestions about possible mechanisms for the creation of rogue waves. These include the combined effects of wind and currents, and the focusing effects associated with the profile of the ocean floor and nearby shorelines. Where rogue waves appear in deep water far from any shore, which they sometimes do, it seems likely that they must evolve through nonlinear interactions within the 'noisy background" of smaller wind-blown waves [4]. Rogue waves have been modeled theoretically, especially by exploiting the special properties of the nonlinear Schrödinger equation. They have been sought experimentally and/or studied in large wave tanks [5], optical systems [6, 7], and superfluid 4He [8]. Our experimental system consists of high intensity second sound (temperature-entropy) waves within a resonant cavity filled with superfluid 4He at 2.1 K. Under steady state conditions, with a constant oscillatory driving force at the resonant frequency, the second sound waves are turbulent and fluxes of energy flow towards both high and low frequencies. It is found that rogue waves appear under the nonequilibrium conditions that prevail shortly after the drive has been

  5. NUCLEAR AND HEAVY ION PHYSICS: Measurement of the astrophysical S factor for the low energy 2H(d,γ)4He reaction

    NASA Astrophysics Data System (ADS)

    Zhou, Jing; Fu, Yuan-Yong; Zhou, Shu-Hua; Xia, Hai-Hong; Li, Cheng-Bo; Meng, Qiu-Ying

    2009-05-01

    The γ-rays and protons from an Ed = 20 keV deuteron beam incident on a D—Ti target were measured. A branching ratio of the 2H(d,γ)4 He reaction versus the 2H(d,p) 3H reaction of Γγ/Γp = (1.06 ± 0.34) × 10-7 has been obtained, and the astrophysical S factor of the 2H(d,γ)4 He reaction at the center of mass energy Ecm approx 7 keV of (6.0 ± 2.4) × 10-6 keV·b was deduced.

  6. Four-body calculation of the first excited state of 4He using a realistic NN interaction: 4He (e, e' ) 4He ( 0+2 ) and the monopole sum rule

    NASA Astrophysics Data System (ADS)

    Hiyama, E.; Gibson, B. F.; Kamimura, M.

    2004-09-01

    4He possesses a second 0+ state; the transition form factor has been measured via inelastic electron scattering. The nature of the 0+2 state’s spatial structure has been controversial. An accurate four-nucleon calculation utilizing a realistic NN force (Argonne V 8' ) plus phenomenological NNN three-body force has been performed for both the 4He ground state and second 0+ state ( Ex =20.21 MeV) using the Gaussian expansion method. The calculated one-body densities and transition density show a significant difference between the states. The resulting impulse approximation transition form factor 4He (e, e' ) 4He ( 0+2 ) agrees with the available data. The overlap of the 0+2 wave function with the trinucleon ground state suggests that the structure is primarily a loosely bound 3N+N system and not a breathing mode. It is found that a major part of the energy-weighted E0 sum rule value is exhausted by nonresonant, low-energy continuum states other than the second 0+ state, in contrast to heavier nuclei where a dominant fraction of the sum-rule limit is exhausted by the second 0+ state because it corresponds to a collective, breathing mode.

  7. Quantum effects in the sorption kinetics of 4He by mesoporous materials

    NASA Astrophysics Data System (ADS)

    Dolbin, A. V.; Khlistyuck, M. V.; Esel'son, V. B.; Gavrilko, V. G.; Vinnikov, N. A.; Basnukaeva, R. M.; Danchuk, V. V.

    2016-02-01

    Sorption and desorption of 4He by a mesoporous silicate material MCM-41 was studied in the temperature range of 1.5-290 K. It was shown that for T = 25-290 K the thermal activation mechanism is dominant in the sorption kinetics of 4He atoms by an MCM-41 sample. Its activation energy was estimated as Ea ≈ 164.8 K. For T = 12-23 K, the diffusion of 4He atoms in the MCM-41 was practically independent of temperature, which typically occurs when the tunnelling mechanism of diffusion dominates over the thermally activated one. A change in the mobility of 4He atoms in MCM-41 channels was observed at T = 6-12 K, which may be indicative of the formation upon cooling (or decay upon heating) of a 4He monolayer and subsequent multilayers on the inner surfaces of the channels. Below 6 K, the diffusion coefficients of 4He are only weakly temperature dependent, which may be attributed to the behavior of quantum 4He liquid in the MCM-41 channels covered with several layers of 4He atoms.

  8. Anisotropic superfluidity of {sup 4}He on a C{sub 36} fullerene molecule

    SciTech Connect

    Park, Sungjin; Kim, Byeongjoon; Kwon, Yongkyung

    2015-09-14

    We have performed path-integral Monte Carlo calculations to study the adsorption of {sup 4}He atoms on two different C{sub 36} isomers with the D{sub 6h} and the D{sub 2d} symmetries. The radial {sup 4}He density distributions reveal layer-by-layer growth with the first layer being located at a distance of ∼5.5 Å from the C{sub 36} molecular center and the second layer at ∼8.3 Å. From the angular density profiles of {sup 4}He, we find different quantum states as the number of {sup 4}He adatoms N varies. For N = 20, we observe commensurate solid structures on both D{sub 6h} and D{sub 2d} isomers, where each of 8 hexagon and 12 pentagon centers of the fullerene surfaces is occupied by a single {sup 4}He atom. The second-layer promotion starts beyond N = 38 on both isomers, where a compressible incommensurate structure is observed on the D{sub 6h} isomer and another commensurate structure on D{sub 2d}. Between N = 20 and N = 38, the {sup 4}He monolayer on D{sub 6h} shows several distinct rings of delocalized {sup 4}He atoms along with strongly anisotropic superfluid responses at low temperatures, while isotropic but weak superfluid responses are observed in the {sup 4}He layer on D{sub 2d}.

  9. Anisotropic superfluidity of (4)He on a C36 fullerene molecule.

    PubMed

    Park, Sungjin; Kim, Byeongjoon; Kwon, Yongkyung

    2015-09-14

    We have performed path-integral Monte Carlo calculations to study the adsorption of (4)He atoms on two different C36 isomers with the D6h and the D2d symmetries. The radial (4)He density distributions reveal layer-by-layer growth with the first layer being located at a distance of ∼5.5 Å from the C36 molecular center and the second layer at ∼8.3 Å. From the angular density profiles of (4)He, we find different quantum states as the number of (4)He adatoms N varies. For N = 20, we observe commensurate solid structures on both D6h and D2d isomers, where each of 8 hexagon and 12 pentagon centers of the fullerene surfaces is occupied by a single (4)He atom. The second-layer promotion starts beyond N = 38 on both isomers, where a compressible incommensurate structure is observed on the D6h isomer and another commensurate structure on D2d. Between N = 20 and N = 38, the (4)He monolayer on D6h shows several distinct rings of delocalized (4)He atoms along with strongly anisotropic superfluid responses at low temperatures, while isotropic but weak superfluid responses are observed in the (4)He layer on D2d. PMID:26374039

  10. Nuclear georeactor origin of oceanic basalt 3He/4He, evidence, and implications

    PubMed Central

    Herndon, J. Marvin

    2003-01-01

    Nuclear georeactor numerical simulation results yield substantial 3He and 4He production and 3He/4He ratios relative to air (RA) that encompass the entire 2-SD (2σ) confidence level range of tabulated measured 3He/4He ratios of basalts from along the global spreading ridge system. Georeactor-produced 3He/4He ratios are related to the extent of actinide fuel consumption at time of production and are high near the end of the georeactor lifetime. Georeactor numerical simulation results and the observed high 3He/4He ratios measured in Icelandic and Hawaiian oceanic basalts indicate that the demise of the georeactor is approaching. Within the present level of uncertainty, one cannot say precisely when georeactor demise will occur, whether in the next century, in a million years, or in a billion years from now. PMID:12615991

  11. {sup 4}He adsorption and superfluid transition on C{sub 60}

    SciTech Connect

    Teizer, W.; Hallock, R.B.; Hebard, A.F.

    1997-10-01

    The authors present adsorption isotherm data of {sup 4}He on C{sub 60} for 1.50 K < T < 1.68 K determined by measurements of the frequency of quartz crystal microbalances (QCM`s) coated with C{sub 60} films. They find a Kosterlitz-Thouless transition with a jump in the areal superfluid density close to predictions. By comparing the adsorbed {sup 4}He on two QCM`s they derive an upper limit for the amount of {sup 4}He intercalated into C{sup 60} at low temperature of 0.05 {sup 4}He atoms per C{sub 60} molecule. The low coverage portion of the adsorption data shows an apparent excess adsorption of {sup 4}He onto the C{sub 60}.

  12. Two-neutron transfer analysis of the 16O(18O,16O)18O reaction

    NASA Astrophysics Data System (ADS)

    Ermamatov, M. J.; Cappuzzello, F.; Lubian, J.; Cubero, M.; Agodi, C.; Carbone, D.; Cavallaro, M.; Ferreira, J. L.; Foti, A.; Garcia, V. N.; Gargano, A.; Lay, J. A.; Lenzi, S. M.; Linares, R.; Santagati, G.; Vitturi, A.

    2016-08-01

    Recently a quantitative description of the two-neutron transfer reaction 12C(18O,16O)14C was performed and the measured cross sections were successfully reproduced [M. Cavallaro et al., Phys. Rev. C 88, 054601 (2013), 10.1103/PhysRevC.88.054601]. This task was accomplished by combining nuclear structure calculations of spectroscopic amplitudes and a full quantum description of the reaction mechanism. Verification of such a theoretical approach to other heavy nuclear systems is mandatory in order to use (18O,16O ) reactions to assess pair configurations in nuclear states. In this work we apply this methodology to the 16O(18O,16O)18O reaction at 84 MeV. Experimental angular distributions for the two-neutron transfer to the ground state and 21+ state of 18O were obtained using the MAGNEX spectrometer at INFN-LNS. The roles of one- and two-step processes are analyzed under the exact finite range coupled reaction channel and the second order distorted wave Born approximation. We conclude that the one-step transfer mechanism is dominant in this system.

  13. Isovector dipole resonances in {sup 4}He and neutrino-heating in supernova

    SciTech Connect

    Nakayama, S.; Matsumoto, E.; Fushimi, K.; Hayami, R.; Suzuki, T.; Yamagata, T.; Akimune, H.; Ikemizu, H.; Fujiwara, M.; Hashimoto, H.; Kawase, K.; Nakanishi, K.; Oota, T.; Yosoi, M.; Greenfield, M. B.; Kudoh, T.; Sagara, K.; Tanaka, M.

    2010-06-01

    We studied transition strengths to isovector dipole resonances (GDR-1-bar , SDR-1-bar , and SDR-2-bar ) in {sup 4}He by using the {sup 4}He({sup 7}Li,{sup 7}Begamma) reaction at 455 MeV and by comparing with shell-model calculations, in order to estimate cross sections of {sup 4}He for reactions induced by neutrinos emitting from a thermalized neutrino-sphere in the type-II supernova. Excitation of the SDR was dominant in the neutrino-heating of {sup 4}He. The {sup 4}He-excitation via neutral-current reactions of nu{sub m}u{sub ,t}au and nu-bar{sub m}u{sub ,t}au was found to be one order of magnitude stronger than that via charged-current reactions of nu{sub e} and nu-bar{sub e}. The total energy-weighted cross section {sub N} for neutrino-induced neutral-current reactions on {sup 4}He was found to amount to about 1.0x10{sup -40} MeVcentre dotcm{sup 2} which is comparable to those used in the previous simulations. The neutrino-heating effect of {sup 4}He is small in the type-II supernova explosion.

  14. Radiogenic 4He as a conservative tracer in buried-valley aquifers

    USGS Publications Warehouse

    Van Der Hoven, S. J.; Wright, R.E.; Carstens, D.A.; Hackley, Keith C.

    2005-01-01

    [1] The accumulation of 4He in groundwater can be a powerful tool in hydrogeologic investigations. However, the use of 4He often suffers from disagreement or uncertainty related to in situ and external sources of 4He. In situ sources are quantified by several methods, while external sources are often treated as calibration parameters in modeling. We present data from direct laboratory measurements of 4He release from sediments and field data of dissolved 4He in the Mahomet Aquifer, a well-studied buried-valley aquifer in central Illinois. The laboratory-derived accumulation rates (0.13-0.91 ??cm3 STP kgwater-1 yr-1) are 1-2 orders of magnitude greater than the accumulation rates based on the U and Th concentrations of the sediments (0.004-0.009 ??cm3 STP kgwater-1 yr -1). The direct measurement of accumulation rates are more consistent with dissolved concentrations of 4He in the groundwater. We suggest that the direct measurement method is applicable in a variety of hydrogeologic settings. The patterns of accumulation of 4He are consistent with the conceptual model of flow in the aquifer based on hydraulic and geochemical evidence and show areas where in situ production and external sources of 4He are dominant. In the southwestern part of the study area, Ne concentrations are less than atmospheric solubility, indicating gases have been lost from the groundwater. Available evidence indicates that the gases are lost as groundwater passes by pockets of CH4 in glacial deposits overlying the aquifer. However, the external flux from the underlying bedrock appears to dominate the accumulation of radiogenic 4He in the aquifer in the southwestern part of the study area, and the loss or gain of helium as groundwater passes through the overlying sediments is minor in comparison. Copyright 2005 by the American Geophysical Union.

  15. Interlayer correlation between two 4He monolayers adsorbed on both sides of α -graphyne

    NASA Astrophysics Data System (ADS)

    Ahn, Jeonghwan; Park, Sungjin; Lee, Hoonkyung; Kwon, Yongkyung

    2015-07-01

    Path-integral Monte Carlo calculations have been performed to study the 4He adsorption on both sides of a single α -graphyne sheet. For investigation of the interlayer correlation between the upper and the lower monolayers of 4He adatoms, the 4He-substrate interaction is described by the sum of the 4He-C interatomic pair potentials for which we use both Lennard-Jones and Yukawa-6 anisotropic potentials. When the lower 4He layer is a C4 /3 commensurate solid, the upper-layer 4He atoms are found to form a kagome lattice structure at a Mott-insulating density of 0.0706 Å-2 and a commensurate solid at an areal density of 0.0941 Å-2 for both substrate potentials. The correlation between upper- and lower-layer pseudospins, which were introduced in Kwon et al. [Phys. Rev. B 88, 201403(R) (2013)], 10.1103/PhysRevB.88.201403 for two degenerate configurations of three 4He atoms in a hexagonal cell, depends on the substrate potential used; with the substrate potential based on the anisotropic Yukawa-6 pair potentials, the Ising pseudospins of both 4He layers are found to be antiparallel to each other whereas the parallel and antiparallel pseudospin alignments between the two 4He layers are nearly degenerate with the Lennard-Jones potentials. This is attributed to the difference in the interlayer distance, which is ˜4 Å with the Yukawa-6 substrate potential but as large as ˜4.8 Å with the Lennard-Jones potential.

  16. Viscosity of liquid {sup 4}He and quantum of circulation: Are they related?

    SciTech Connect

    L’vov, Victor S. E-mail: skrbek@fzu.cz; Skrbek, Ladislav E-mail: skrbek@fzu.cz; Sreenivasan, Katepalli R. E-mail: skrbek@fzu.cz

    2014-04-15

    In the vicinity of the superfluid transition in liquid {sup 4}He, we explore the relation between two apparently unrelated physical quantities—the kinematic viscosity, ν, in the normal state and the quantum of circulation, κ, in the superfluid state. The model developed here leads to the simple relationship ν ≈ κ/6, and links the classical and quantum flow properties of liquid {sup 4}He. We critically examine available data relevant to this relation and find that the prediction holds well at the saturated vapor pressure. Additionally, we predict the kinematic viscosity for liquid {sup 4}He along the λ-line at negative pressures.

  17. Comment on ''Few-atom /sup 3/He--/sup 4/He mixed molecules''

    SciTech Connect

    Harada, M.

    1983-02-15

    It is pointed out that a recent work by Nakaichi et al. on few-atom /sup 3/He--/sup 4/He mixed molecules is based on incorrect values of THETA/sup 2//M/sub 3/ and THETA/sup 2//M/sub 4/, where M/sub 3/ and M/sub 4/ are the masses of the /sup 3/He and /sup 4/He atoms. This is shown to affect their conclusion on the /sup 3/He(/sup 4/He)/sub 2/ system seriously.

  18. Development of a thermodynamic model for a cold cycle 3He-4He dilution refrigerator

    NASA Astrophysics Data System (ADS)

    Mueller, B. W.; Miller, F. K.

    2016-10-01

    A thermodynamic model of a 3He-4He cold cycle dilution refrigerator with no actively-driven mechanical components is developed and investigated. The refrigerator employs a reversible superfluid magnetic pump, passive check valves, a phase separation chamber, and a series of recuperative heat exchangers to continuously circulate 3He-4He and maintain a 3He concentration gradient across the mixing chamber. The model predicts cooling power and mixing chamber temperature for a range of design and operating parameters, allowing an evaluation of feasibility for potential 3He-4He cold cycle dilution refrigerator prototype designs. Model simulations for a prototype refrigerator design are presented.

  19. Unusual Doppler effect in superfluid and nonanalyticity of {sup 4}He-{sup 3}He hydrodynamics

    SciTech Connect

    Nepomnyashchy, Y.A.; Gov, N.; Mann, A.

    1995-08-01

    The authors investigate the influence of {sup 3}He admixture on the Doppler shift of different sounds in superfluid {sup 4}He with internal motion. This influence proves to be very strong in the whole region of the nontrivial temperature behavior of the Doppler shift and implies in particular an unexpected amplification of certain Doppler anomalies. They explain origin of the features of the internal Doppler effect in pure {sup 4}He and {sup 4}He-{sup 3}He mixture and notice an interesting peculiarity of the {sup 4}He-{sup 3}He two-fluid hydrodynamics: its nonanalyticity at low temperature and small {sup 3}He concentration: T{yields}0, X{yields}0.

  20. New Phenomenon of the Hysteresis of 4He in Vycor Glass

    NASA Astrophysics Data System (ADS)

    Jin, Xin; Xu, Xiaonong; Yan, Yong; A, L. Thomson; D, F. Brewer; S, Haynes; N, Sharma

    1992-02-01

    The low temperature part of hysteresis curves of the freezing and melting processes of 4He in vycor glass with the lowest temperature 0.4K were measured, as the pressure ranged from 36.45 to 55.18 (105 Pa). Some novel characteristics of these curves were observed in such high temperature and pressure range. They may result from the existence of superfluid 4He.

  1. Resonances in (11)C observed in the (4)He((7)Be, alpha)(7)Be and (4)He((7)Be, p)(10)B reactions

    SciTech Connect

    Freer, M.; Ashwood, N. I.; Curtis, N.; Malcolm, J.; Munoz-Britton, T.; Price, D.; Wheldon, C.; Achouri, N. L.; Demaret, P.; Bardayan, Daniel W; Pain, Steven D; Brown, S.; Catford, W.; Harlin, Christopher W; Thomas, J. S.; Wilson, G.; Chipps, K.; Milin, M.; Raabe, R.; Soic, N.

    2012-01-01

    Measurements of the {sup 4}He({sup 7}Be,{alpha}){sup 7}Be and {sup 4}He({sup 7}Be,p){sup 10}B reactions were performed using {sup 7}Be beam energies of 7.1 and 23 MeV and a helium-4 target, employing the thick target technique. Resonances were observed between E{sub x}({sup 11}C) = 8.6 to 13.8 MeV. An R-matrix analysis was performed to characterize the spins and partial widths. This analysis showed that the observed sequence of states was consistent with that found for {sup 7}Li + {alpha} resonant scattering populating resonances in {sup 11}B. A comparison of the proposed partial widths for decay with the Wigner limit indicates that several of the states are associated with cluster-like structures.

  2. New light on the intriguing history of superfluidity in liquid (4)He.

    PubMed

    Griffin, Allan

    2009-04-22

    Surprisingly, it was 30 years after the first liquefaction of (4)He in 1908 that the discovery that liquid (4)He is not just a 'cold' liquid was made. Below T = 2.18 K, it is a 'quantum' liquid which exhibits spectacular macroscopic quantum behaviour that can be seen with the naked eye. Since the observation of superfluidity in liquid (4)He is one of the greatest discoveries in modern physics, we present a day-to-day chronology of the tangled events which preceded the seminal discovery of zero viscosity in 1938 by Kapitza in Moscow and by Allen and Misener in Cambridge. On the theory side, London argued in 1938 that the microscopic basis for this new superfluid phase was the forgotten phenomenon of Bose-Einstein condensation (BEC) first suggested by Einstein in 1925. In 1941, Landau developed a very successful theory of superfluid (4)He, but it was not anchored in a microscopic theory of interacting atoms. It took another 20 years for theorists to unify the two seemingly different theories of Landau and London. Experiments on trapped superfluid atomic gases since 1995 have shone new light on superfluid (4)He. In the mid-1930s, London had emphasized that superconductivity in metals and superfluidity in liquid (4)He were similar. Experiments on trapped two-component Fermi gases in the last five years have shown that a Bose condensate is indeed the basis of both of these superfluid phases. This confirms the now famous Bardeen-Cooper-Schrieffer-BEC crossover scenario developed for superfluidity by Leggett and Nozières in the early 1980s but largely ignored until a few years ago. The study of superfluid (4)He will increasingly overlap with strongly interacting dilute quantum gases, perhaps opening up a new era of research on this most amazing liquid.

  3. New light on the intriguing history of superfluidity in liquid 4He

    NASA Astrophysics Data System (ADS)

    Griffin, Allan

    2009-04-01

    Surprisingly, it was 30 years after the first liquefaction of 4He in 1908 that the discovery that liquid 4He is not just a 'cold' liquid was made. Below T = 2.18 K, it is a 'quantum' liquid which exhibits spectacular macroscopic quantum behaviour that can be seen with the naked eye. Since the observation of superfluidity in liquid 4He is one of the greatest discoveries in modern physics, we present a day-to-day chronology of the tangled events which preceded the seminal discovery of zero viscosity in 1938 by Kapitza in Moscow and by Allen and Misener in Cambridge. On the theory side, London argued in 1938 that the microscopic basis for this new superfluid phase was the forgotten phenomenon of Bose-Einstein condensation (BEC) first suggested by Einstein in 1925. In 1941, Landau developed a very successful theory of superfluid 4He, but it was not anchored in a microscopic theory of interacting atoms. It took another 20 years for theorists to unify the two seemingly different theories of Landau and London. Experiments on trapped superfluid atomic gases since 1995 have shone new light on superfluid 4He. In the mid-1930s, London had emphasized that superconductivity in metals and superfluidity in liquid 4He were similar. Experiments on trapped two-component Fermi gases in the last five years have shown that a Bose condensate is indeed the basis of both of these superfluid phases. This confirms the now famous Bardeen-Cooper-Schrieffer-BEC crossover scenario developed for superfluidity by Leggett and Nozières in the early 1980s but largely ignored until a few years ago. The study of superfluid 4He will increasingly overlap with strongly interacting dilute quantum gases, perhaps opening up a new era of research on this most amazing liquid.

  4. Incomplete fusion in 16O+159Tb

    NASA Astrophysics Data System (ADS)

    Sharma, Vijay R.; Singh, Pushpendra P.; Shuaib, Mohd.; Yadav, Abhishek; Bala, Indu; Sharma, Manoj K.; Gupta, S.; Singh, D. P.; Kumar, R.; Muralithar, S.; Singh, R. P.; Singh, B. P.; Prasad, R.; Bhowmik, R. K.

    2016-02-01

    In heavy-ion induced reactions, incomplete fusion (ICF) has been found to be a process of greater importance and of distinct nature even at slightly above the barrier energies where complete fusion (CF) is supposed to be dominant. However, the studies are limited to a few projectile target combinations only. To confirm the distinctly different decay patterns observed in case of CF and ICF residues, and to understand the role of high ℓ-values in the onset of ICF, a particle-γ-coincidence technique has been employed to measure spin-distributions and feeding intensity profiles of CF and ICF residues populated via xn / pxn / αxn-channels in 16O+159Tb interactions at Elab ≈ 83.5 ± 1.5, 88.5 ± 1.5, 93.5 ± 1.5 and 97.6 ± 1.4 MeV. The Gamma Detector Array and the Charged Particles Detector Array have been used to detect prompt γ-rays in coincidence with charged particles (p and α). CF-α and ICF-α channels have been identified from backward (B)- and forward (F)-α-gated-γ-spectra, respectively. Reaction dependent decay patterns (thus, the feeding intensity profiles) have been observed in different α emitting channels. The CF channels are found to be widely populated and strongly fed over a broad spin range. In case of ICF-α channels, narrow range feeding was observed only for high-spin states or the low spin states were not populated. The mean ℓ-values involved in the production of ICF- αxn-channels are found to be higher than those involved in the production of CF- αxn-channels associated with fusion-evaporation reactions.

  5. Heavy-ion versus {sup 3}He/{sup 4}He fusion-fission reactions: Angular momentum dependence of dissipation in nuclear fission

    SciTech Connect

    Ye, W.

    2011-09-15

    The stochastic Langevin model is employed to study dissipation properties in fission in the {sup 16}O + {sup 181}Ta {yields}{sup 197}Tl system by analyzing prescission neutron yields measured in this reaction. It has been found that the {sup 197}Tl nuclei undergo fission that is not in accordance with the standard Bohr-Wheeler statistical theory. A detailed comparison with previously published work in which fission excitation functions measured in {sup 3,4}He + {sup 197}Au {yields}{sup 200,201}Tl are shown to be in excellent agreement with the fission width formula predicted by the traditional models of nuclear fission suggests that nuclear dissipation strength may have an angular momentum dependence in addition to the known deformation and temperature dependence. Implications for the basic understanding of the observed abnormal rise in prescission particles at high energy and the need for further experimental confirmations are discussed.

  6. Mineralogy of IDPs with Known 4He and Trace Element Contents

    NASA Astrophysics Data System (ADS)

    Klock, W.; Flynn, G. J.; Sutton, S. R.; Nier, A. O.

    1992-07-01

    Interplanetary Dust Particles (IDPs) collected in the atmosphere are a very special source of information about solar system objects like asteroids and comets. Suggested IDP properties indicative of their origins include amounts of 4He and 4He release temperatures (Nier and Schlutter 1990, 1992), solar flare track densities (Sandford and Bradley 1989), and trace element abundances (Flynn et al. 1992). Recently Flynn et al. (1992) suggested that Zn depletions of IDPs are indicative of heating in the atmosphere. On the average, asteroidal particles experience less heating than cometary particles (Flynn 1989). Nier and Schlutter (1992) showed that 4He release temperatures of individual IDPs vary from 420 C up to more than 800 C. Presently it is not clear if variations of 4He contents are a result of the original mineral compositions, and therefore source of individual IDPs, or if they are mainly affected by atmospheric entry heating. We studied the mineralogy of IDPs having variable amounts of 4He. Some of the particles were analyzed by SXRF for volatile trace elements. The particles in Table 1 are ordered according to their amount of 4He. High 4He contents (>11.0 x 1O^-11 cm^3) are found among particles characterized by their porous texture and occurrence of unequilibrated mineral phases. Particles of this group contain abundant glass, solar flare tracks are preserved and have chondritic Zn abundances. Among the 13 particles having low 4He contents six particles contain magnetite crystals that formed by atmospheric entry heating. Three magnetite-bearing particles are low in Zn. Though high in Zn, due to a Zn-bearing iron-sulfide in the center, L2005C19 is a heated particle. L2005A8 is texturally similar to other heated particles, but magnetites were so far not identified. According to Rietmeijer and Mackinnon (1985), particle W7029*A was not heated above 315 C and this explains its chondritic Zn level at a low amount of 4He. Three hydrated IDPs have low 4He contents

  7. Control of the wetting properties of 4He crystals in superfluid

    NASA Astrophysics Data System (ADS)

    Takahashi, T.; Minezaki, H.; Suzuki, A.; Obara, K.; Itaka, K.; Nomura, R.; Okuda, Y.

    2016-05-01

    To investigate whether it is possible to control the wetting of 4He crystals on a wall in superfluid, the contact angles of 4He crystals were measured on rough and smooth walls at very low temperatures. A rough wall was prepared in a simple manner in which a commercially available coating agent for car mirrors, which makes the glass surface superhydrophobic, was used to coat a glass plate. The contact angles of 4He crystals were increased by approximately 10° on the rough wall coated with the agent. Therefore, the increase in the repellency of 4He crystals in superfluid was demonstrated to be possible on a very rough surface. The enhancement of the contact angles and a scanning electron microscopy image of the coated surface both suggest that a Cassie-Baxter state of 4He crystals was realized on the surface; the crystals did not have full contact with the wall, but entrapped superfluid was present beneath the crystals in the hollow parts of the rough wall.

  8. Control of the wetting properties of ^{4}He crystals in superfluid.

    PubMed

    Takahashi, T; Minezaki, H; Suzuki, A; Obara, K; Itaka, K; Nomura, R; Okuda, Y

    2016-05-01

    To investigate whether it is possible to control the wetting of ^{4}He crystals on a wall in superfluid, the contact angles of ^{4}He crystals were measured on rough and smooth walls at very low temperatures. A rough wall was prepared in a simple manner in which a commercially available coating agent for car mirrors, which makes the glass surface superhydrophobic, was used to coat a glass plate. The contact angles of ^{4}He crystals were increased by approximately 10^{∘} on the rough wall coated with the agent. Therefore, the increase in the repellency of ^{4}He crystals in superfluid was demonstrated to be possible on a very rough surface. The enhancement of the contact angles and a scanning electron microscopy image of the coated surface both suggest that a Cassie-Baxter state of ^{4}He crystals was realized on the surface; the crystals did not have full contact with the wall, but entrapped superfluid was present beneath the crystals in the hollow parts of the rough wall.

  9. On the origin of (4)He and (40)Ar in natural gold

    NASA Technical Reports Server (NTRS)

    Eugster, O.; Hofmann, B.; Niedermann, S.; Thalmann, CH.

    1993-01-01

    In a first report on our investigations of noble gases in native gold we demonstrated that placer gold contains an excess of radiogenic (4)He and (40)Ar relative to the concentrations expected from in situ decay of U, Th, and K, respectively, during the geologic age of about 30 Ma of the samples. We also showed that the U/Th-(4)He age of 36 Ma of vein-type gold from the Southern Alps agrees with its K-Ar formation age derived from associated muscovite and biotite. We now studied the question of the origin of the (4)He and (40)Ar excesses of placer gold. We conclude that gold contains two components of noble gases, a low-temperature component from fluid inclusions or phases which release noble gases at less than 800 C and a high-temperature component released when gold melts (1064 C). In some samples extremely high U and K concentrations or an unreasonably high formation age would be required to explain the observed (4)He abundances. Thus, trapped (4)He and (40)Ar must be present in gold.

  10. High-resolution measurement of absolute {alpha}-decay widths in {sup 16}O

    SciTech Connect

    Wheldon, C.; Ashwood, N. I.; Barr, M.; Curtis, N.; Freer, M.; Kokalova, Tz.; Malcolm, J. D.; Spencer, S. J.; Ziman, V. A.; Faestermann, Th.; Kruecken, R.; Wirth, H.-F.; Hertenberger, R.; Lutter, R.; Bergmaier, A.

    2011-06-15

    By using a large-acceptance position-sensitive silicon detector array in coincidence with the high-resolution Munich Q3D spectrograph, unambiguous measurements have been made of the absolute {alpha}-particle decay widths from excited states in {sup 16}O* in the energy range 13.85 to 15.87 MeV. Carbon targets have been bombarded with 42-MeV {sup 6}Li beams to induce {sub 6}{sup 12}C({sub 3}{sup 6}Li, d){sub 8}{sup 16}O* reactions. The deuteron ejectiles were measured in the Q3D and the results gated by {sup 4}He+{sup 12}C breakup products detected in the silicon array, the efficiency of which was modeled using Monte Carlo simulations. By comparing total population and breakup-gated spectra, the following absolute {alpha}-decay widths have been measured with high resolution: {Gamma}{sub {alpha}}0/{Gamma}{sub tot} = 0.87{+-}0.11 (13.980 MeV), 1.04{+-}0.15 (14.302 MeV), 0.92{+-}0.10 (14.399 MeV), 0.59{+-}0.04 (14.815 MeV), 0.88{+-}0.18 (15.785 MeV), and {Gamma}{sub {alpha}}1/{Gamma}{sub tot}=1.14{+-}0.08 (14.660 MeV), 0.46{+-}0.06 (14.815 MeV).

  11. Green's function theory for the Cheng-Schick model of 3He-4He mixtures

    NASA Astrophysics Data System (ADS)

    Siemann, R. P.; Boukahil, A.; Huber, D. L.

    2014-08-01

    In this paper, we outline a theory for the thermodynamic properties of 3He-4He mixtures in the neighborhood of the critical line and the tricritical point (TCP). The theory utilizes the Cheng-Schick (CS) lattice gas model where both the 3He and 4He atoms are treated as quantum particles on a lattice. The analysis is based on Green's function approach. Results are presented for the ordering susceptibility and the thermal averages of the occupation numbers of 3He and 4He atoms. We derive a self-consistent equation for the ordering susceptibility and use it to calculate the critical line and locate the TCP. Our findings are compared with the predictions obtained from high temperature series expansions, mean field theory and the random phase approximation (RPA).

  12. Upper bound on parity-violating neutron spin rotation in {sup 4}He

    SciTech Connect

    Snow, W. M.; Luo, D.; Walbridge, S. B.; Crawford, B. E.; Gan, K.; Micherdzinska, A. M.; Opper, A. K.; Heckel, B. R.; Swanson, H. E.; Sharapov, E. I.; Zhumabekova, V.

    2011-02-15

    We report an upper bound on parity-violating neutron spin rotation in {sup 4}He. This experiment is the most sensitive search for neutron-weak optical activity yet performed and represents a significant advance in precision in comparison to past measurements in heavy nuclei. The experiment was performed at the NG-6 slow-neutron beamline at the National Institute of Standards and Technology (NIST) Center for Neutron Research. Our result for the neutron spin rotation angle per unit length in {sup 4}He is d{phi}/dz=[+1.7{+-}9.1(stat.){+-}1.4(sys.)]x10{sup -7} rad/m. The statistical uncertainty is smaller than current estimates of the range of possible values of d{phi}/dz in n+{sup 4}He.

  13. Extracting the spectral function of 4He from a relativistic plane-wave treatment

    NASA Astrophysics Data System (ADS)

    Abu-Raddad, L. J.; Piekarewicz, J.

    2001-12-01

    The spectral function of 4He is extracted from a plane-wave approximation to the (e,e'p) reaction using a fully relativistic formalism. We take advantage of both an algebraic ``trick'' and a general relativistic formalism for quasifree processes developed earlier to arrive at transparent, analytical expressions for all quasifree (e,e'p) observables. An observable is identified for the clean and model-independent extraction of the spectral function. Our simple relativistic plane-wave calculations provide baseline predictions for the recently measured, but not yet fully analyzed, momentum distribution of 4He by the A1 Collaboration from Mainz. Yet in spite of its simplicity, our approach predicts momentum distributions for 4He that rival some of the best nonrelativistic calculations to date. Finally, we highlight some of the challenges and opportunities that remain, both theoretically and experimentally, in the extraction of quasifree observables.

  14. Calibration Technique for Superfluid 4He Weak-Link Cells Based on the Fountain Effect

    SciTech Connect

    Hoskinson, E.; Packard, R. E.

    2006-09-07

    Studies of superfluid 4He weak-links require calibration constants which permit the determination of the pressure and temperature differences which drive Josephson oscillations. We describe a technique for calibrating 4He weak-link cells in which a heater is used to induce fountain pressures detected by the deflection of a diaphragm. The technique determines the diaphragm spring constant, the inner cell volume, and the thermal conductance of the inner cells walls. This information is used to convert the measured deflection of the diaphragm into the total chemical potential difference across the weak link.

  15. JLab measurement of the 4He charge form factor at large momentum transfers.

    PubMed

    Camsonne, A; Katramatou, A T; Olson, M; Sparveris, N; Acha, A; Allada, K; Anderson, B D; Arrington, J; Baldwin, A; Chen, J-P; Choi, S; Chudakov, E; Cisbani, E; Craver, B; Decowski, P; Dutta, C; Folts, E; Frullani, S; Garibaldi, F; Gilman, R; Gomez, J; Hahn, B; Hansen, J-O; Higinbotham, D W; Holmstrom, T; Huang, J; Iodice, M; Jiang, X; Kelleher, A; Khrosinkova, E; Kievsky, A; Kuchina, E; Kumbartzki, G; Lee, B; LeRose, J J; Lindgren, R A; Lott, G; Lu, H; Marcucci, L E; Margaziotis, D J; Markowitz, P; Marrone, S; Meekins, D; Meziani, Z-E; Michaels, R; Moffit, B; Norum, B; Petratos, G G; Puckett, A; Qian, X; Rondon, O; Saha, A; Sawatzky, B; Segal, J; Shabestari, M; Shahinyan, A; Solvignon, P; Subedi, R R; Suleiman, R; Sulkosky, V; Urciuoli, G M; Viviani, M; Wang, Y; Wojtsekhowski, B B; Yan, X; Yao, H; Zhang, W-M; Zheng, X; Zhu, L

    2014-04-01

    The charge form factor of 4He has been extracted in the range 29  fm(-2) ≤ Q2 ≤ 77  fm(-2) from elastic electron scattering, detecting 4He recoil nuclei and electrons in coincidence with the high resolution spectrometers of the Hall A Facility of Jefferson Lab. The measurements have uncovered a second diffraction minimum for the form factor, which was predicted in the Q2 range of this experiment. The data are in qualitative agreement with theoretical calculations based on realistic interactions and accurate methods to solve the few-body problem. PMID:24745410

  16. Using the surface tension to estimate the condensate density of superfluid /sup 4/He

    SciTech Connect

    Campbell, L.J.

    1983-01-01

    Distortion of the condensate wavefunction at the free surface of superfluid /sup 4/He contributes to the surface tension in proportion to the condensate fraction n/sub 0/(T). Using this to resolve the present discrepancy between the measured and predicted temperature dependencies of the surface tension gives n/sub 0/(T) in good agreement with results from neutron and x-ray scattering measurements. This picture is also consistent with the measured /sup 3/He-/sup 4/He interfacial tension.

  17. Indirect Study of the 16O+16O Fusion Reaction Toward Stellar Energies by the Trojan Horse Method

    NASA Astrophysics Data System (ADS)

    Hayakawa, S.; Spitaleri, C.; Burtebayev, N.; Aimaganbetov, A.; Figuera, P.; Fisichella, M.; Guardo, G. L.; Igamov, S.; Indelicato, I.; Kiss, G.; Kliczewski, S.; La Cognata, M.; Lamia, L.; Lattuada, M.; Piasecki, E.; Rapisarda, G. G.; Romano, S.; Sakuta, S. B.; Siudak, R.; Trzcińska, A.; Tumino, A.; Urkinbayev, A.

    2016-05-01

    The 16O+16O fusion reaction is important in terms of the explosive oxygen burning process during late evolution stage of massive stars as well as understanding of the mechanism of low-energy heavy-ion fusion reactions. We aim to determine the excitation function for the most major exit channels, α+28Si and p+31P, toward stellar energies indirectly by the Trojan Horse Method via the 16O(20Ne, α28Si)α and 16O(20Ne, p31P)α three-body reactions. We report preliminary results involving reaction identification, and determination of the momentum distribution of α-16O intercluster motion in the projectile 20Ne nucleus.

  18. Equilibrium shape of 4He crystal under zero gravity below 200 mK

    PubMed Central

    Takahashi, Takuya; Ohuchi, Haruka; Nomura, Ryuji; Okuda, Yuichi

    2015-01-01

    Equilibrium crystal shape is the lowest energy crystal shape that is hardly realized in ordinary crystals because of their slow relaxation. 4He quantum crystals in a superfluid have been expected as unique exceptions that grow extremely fast at very low temperatures. However, on the ground, gravity considerably deforms the crystals and conceals the equilibrium crystal shape, and thus, gravity-free environment is needed to observe the equilibrium shape of 4He. We report the relaxation processes of macroscopic 4He crystals in a superfluid below 200 mK under zero gravity using a parabolic flight of a jet plane. When gravity was removed from a gravity-flattened 4He crystal, the crystal rapidly transformed into a shape with flat surfaces. Although the relaxation processes were highly dependent on the initial condition, the crystals relaxed to a nearly homothetic shape in the end, indicating that they were truly in an equilibrium shape minimizing the interfacial free energy. Thanks to the equilibrium shape, we were able to determine the Wulff’s origin and the size of the c-facet together with the vicinal surface profile next to the c-facet. The c-facet size was extremely small in the quantum crystals, and the facet-like flat surfaces were found to be the vicinal surfaces. At the same time, the interfacial free energy of the a-facet and s-facet was also obtained. PMID:26601315

  19. ^4He Crystals in Reduced Gravity Obtained by Parabolic Flights of a Jet Plane

    NASA Astrophysics Data System (ADS)

    Takahashi, Takuya; Nomura, Ryuji; Okuda, Yuichi

    2016-11-01

    ^4He crystals usually sink to the bottom of the container in a superfluid and are deformed into a flat shape by gravity when their size is much larger than the capillary length of 1 mm. When gravity is reduced to zero, the capillary length diverges and the gravity-flattened crystals are expected to relax into an equilibrium crystal shape determined by the interfacial free energy at low enough temperatures where the relaxation time is very short. We performed a reduced gravity experiment on ^4He crystals at ultralow temperatures by developing a specially designed ^3He-^4He dilution refrigerator compatible with the experimental restrictions in a small jet plane. ^4He crystals relaxed to the equilibrium crystal shape below 600 mK during a reduced gravity period of 20 s produced by a parabolic flight. The equilibrium crystal shape, however, was metastable in most cases, governed by the boundary conditions imposed by the wall. Utilizing acoustic radiation pressure, we deformed the crystal enough to allow it to escape from the metastable shape below 150 mK. After this large deformation, the crystal relaxed to a shape completely different from its initial shape, showing three types of facets, viz., c-, a-, and s-facets, which was concluded to be the lowest energy equilibrium shape.

  20. Phase-space analysis of convection in a /sup 3/He - superfluid /sup 4/He solution

    SciTech Connect

    Haucke, H.; Maeno, Y.

    1982-01-01

    Observations have been made on thermal convection below 1K in a dilute solution of /sup 3/He in superfluid /sup 4/He contained in a cylindrical cell of aspect ratio GAMMA = 1.20. Complicated oscillatory phenomena were observed with a high degree of reproducibility using two temperature sensors. Phase-space analysis suggests a description in terms of strange-attractor dynamics.

  1. Third sound and stability of 3He-4He mixture films

    SciTech Connect

    Anderson, R. H.; Krotscheck, E.; Miller, M. D.

    2006-09-07

    We study third sound and the interaction between 3He adatoms in two thin 3He-4He mixture films from a first-principles, microscopic theory. Utilizing the variational, hypernetted-chain Euler-Lagrange (HNC-EL) theory as applied to inhomogeneous boson systems, we calculate chemical potentials for both the 4He superfluid film and the physisorbed 3He. Numerical density derivatives of the chemical potentials lead to the sought-after third sound speeds that clearly reflect a layered structure of at least seven oscillations. In this paper, we report third sound on model substrates: Nuclepore, and sodium. We find that the effect of the 3He depends sensitively on the particular 4He film coverage. Our most important result is that, with the addition of 3He, the third sound speed can either increase or decrease. In fact, in some regimes, the added 3He destabilizes the film and can drive ''layering transitions'', leading to fairly complicated geometric structures of the film in which the outermost layer is predicted to consist of phase-separated regions of 3He and 4He.

  2. Equilibrium shape of (4)He crystal under zero gravity below 200 mK.

    PubMed

    Takahashi, Takuya; Ohuchi, Haruka; Nomura, Ryuji; Okuda, Yuichi

    2015-10-01

    Equilibrium crystal shape is the lowest energy crystal shape that is hardly realized in ordinary crystals because of their slow relaxation. (4)He quantum crystals in a superfluid have been expected as unique exceptions that grow extremely fast at very low temperatures. However, on the ground, gravity considerably deforms the crystals and conceals the equilibrium crystal shape, and thus, gravity-free environment is needed to observe the equilibrium shape of (4)He. We report the relaxation processes of macroscopic (4)He crystals in a superfluid below 200 mK under zero gravity using a parabolic flight of a jet plane. When gravity was removed from a gravity-flattened (4)He crystal, the crystal rapidly transformed into a shape with flat surfaces. Although the relaxation processes were highly dependent on the initial condition, the crystals relaxed to a nearly homothetic shape in the end, indicating that they were truly in an equilibrium shape minimizing the interfacial free energy. Thanks to the equilibrium shape, we were able to determine the Wulff's origin and the size of the c-facet together with the vicinal surface profile next to the c-facet. The c-facet size was extremely small in the quantum crystals, and the facet-like flat surfaces were found to be the vicinal surfaces. At the same time, the interfacial free energy of the a-facet and s-facet was also obtained.

  3. Lieb-Liniger-like model of quantum solvation in CO-(4)HeN clusters.

    PubMed

    Farrelly, D; Iñarrea, M; Lanchares, V; Salas, J P

    2016-05-28

    Small (4)He clusters doped with various molecules allow for the study of "quantum solvation" as a function of cluster size. A peculiarity of quantum solvation is that, as the number of (4)He atoms is increased from N = 1, the solvent appears to decouple from the molecule which, in turn, appears to undergo free rotation. This is generally taken to signify the onset of "microscopic superfluidity." Currently, little is known about the quantum mechanics of the decoupling mechanism, mainly because the system is a quantum (N + 1)-body problem in three dimensions which makes computations difficult. Here, a one-dimensional model is studied in which the (4)He atoms are confined to revolve on a ring and encircle a rotating CO molecule. The Lanczos algorithm is used to investigate the eigenvalue spectrum as the number of (4)He atoms is varied. Substantial solvent decoupling is observed for as few as N = 5 (4)He atoms. Examination of the Hamiltonian matrix, which has an almost block diagonal structure, reveals increasingly weak inter-block (solvent-molecule) coupling as the number of (4)He atoms is increased. In the absence of a dopant molecule the system is similar to a Lieb-Liniger (LL) gas and we find a relatively rapid transition to the LL limit as N is increased. In essence, the molecule initially-for very small N-provides a central, if relatively weak, attraction to organize the cluster; as more (4)He atoms are added, the repulsive interactions between the identical bosons start to dominate as the solvation ring (shell) becomes more crowded which causes the molecule to start to decouple. For low N, the molecule pins the atoms in place relative to itself; as N increases the atom-atom repulsion starts to dominate the Hamiltonian and the molecule decouples. We conclude that, while the notion of superfluidity is a useful and correct description of the decoupling process, a molecular viewpoint provides complementary insights into the quantum mechanism of the transition from a

  4. Lieb-Liniger-like model of quantum solvation in CO-4HeN clusters

    NASA Astrophysics Data System (ADS)

    Farrelly, D.; Iñarrea, M.; Lanchares, V.; Salas, J. P.

    2016-05-01

    Small 4He clusters doped with various molecules allow for the study of "quantum solvation" as a function of cluster size. A peculiarity of quantum solvation is that, as the number of 4He atoms is increased from N = 1, the solvent appears to decouple from the molecule which, in turn, appears to undergo free rotation. This is generally taken to signify the onset of "microscopic superfluidity." Currently, little is known about the quantum mechanics of the decoupling mechanism, mainly because the system is a quantum (N + 1)-body problem in three dimensions which makes computations difficult. Here, a one-dimensional model is studied in which the 4He atoms are confined to revolve on a ring and encircle a rotating CO molecule. The Lanczos algorithm is used to investigate the eigenvalue spectrum as the number of 4He atoms is varied. Substantial solvent decoupling is observed for as few as N = 5 4He atoms. Examination of the Hamiltonian matrix, which has an almost block diagonal structure, reveals increasingly weak inter-block (solvent-molecule) coupling as the number of 4He atoms is increased. In the absence of a dopant molecule the system is similar to a Lieb-Liniger (LL) gas and we find a relatively rapid transition to the LL limit as N is increased. In essence, the molecule initially—for very small N—provides a central, if relatively weak, attraction to organize the cluster; as more 4He atoms are added, the repulsive interactions between the identical bosons start to dominate as the solvation ring (shell) becomes more crowded which causes the molecule to start to decouple. For low N, the molecule pins the atoms in place relative to itself; as N increases the atom-atom repulsion starts to dominate the Hamiltonian and the molecule decouples. We conclude that, while the notion of superfluidity is a useful and correct description of the decoupling process, a molecular viewpoint provides complementary insights into the quantum mechanism of the transition from a molecular

  5. Lieb-Liniger-like model of quantum solvation in CO-(4)HeN clusters.

    PubMed

    Farrelly, D; Iñarrea, M; Lanchares, V; Salas, J P

    2016-05-28

    Small (4)He clusters doped with various molecules allow for the study of "quantum solvation" as a function of cluster size. A peculiarity of quantum solvation is that, as the number of (4)He atoms is increased from N = 1, the solvent appears to decouple from the molecule which, in turn, appears to undergo free rotation. This is generally taken to signify the onset of "microscopic superfluidity." Currently, little is known about the quantum mechanics of the decoupling mechanism, mainly because the system is a quantum (N + 1)-body problem in three dimensions which makes computations difficult. Here, a one-dimensional model is studied in which the (4)He atoms are confined to revolve on a ring and encircle a rotating CO molecule. The Lanczos algorithm is used to investigate the eigenvalue spectrum as the number of (4)He atoms is varied. Substantial solvent decoupling is observed for as few as N = 5 (4)He atoms. Examination of the Hamiltonian matrix, which has an almost block diagonal structure, reveals increasingly weak inter-block (solvent-molecule) coupling as the number of (4)He atoms is increased. In the absence of a dopant molecule the system is similar to a Lieb-Liniger (LL) gas and we find a relatively rapid transition to the LL limit as N is increased. In essence, the molecule initially-for very small N-provides a central, if relatively weak, attraction to organize the cluster; as more (4)He atoms are added, the repulsive interactions between the identical bosons start to dominate as the solvation ring (shell) becomes more crowded which causes the molecule to start to decouple. For low N, the molecule pins the atoms in place relative to itself; as N increases the atom-atom repulsion starts to dominate the Hamiltonian and the molecule decouples. We conclude that, while the notion of superfluidity is a useful and correct description of the decoupling process, a molecular viewpoint provides complementary insights into the quantum mechanism of the transition from a

  6. Search for supersolidity in solid 4He using multiple-mode torsional oscillators

    NASA Astrophysics Data System (ADS)

    Eyal, Anna; Mi, Xiao; Talanov, Artem V.; Reppy, John D.

    2016-06-01

    In 2004, Kim and Chan (KC) reported a decrease in the period of torsional oscillators (TO) containing samples of solid 4He, as the temperature was lowered below 0.2 K [Kim E, Chan MHW (2004) Science 305(5692):1941-1944]. These unexpected results constituted the first experimental evidence that the long-predicted supersolid state of solid 4He may exist in nature. The KC results were quickly confirmed in a number of other laboratories and created great excitement in the low-temperature condensed-matter community. Since that time, however, it has become clear that the period shifts seen in the early experiments can in large part be explained by an increase in the shear modulus of the 4He solid identified by Day and Beamish [Day J, Beamish J (2007) Nature 450(7171):853-856]. Using multiple-frequency torsional oscillators, we can separate frequency-dependent period shifts arising from changes in the elastic properties of the solid 4He from possible supersolid signals, which are expected to be independent of frequency. We find in our measurements that as the temperature is lowered below 0.2 K, a clear frequency-dependent contribution to the period shift arising from changes in the 4He elastic properties is always present. For all of the cells reported in this paper, however, there is always an additional small frequency-independent contribution to the total period shift, such as would be expected in the case of a transition to a supersolid state.

  7. Search for supersolidity in solid 4He using multiple-mode torsional oscillators

    NASA Astrophysics Data System (ADS)

    Eyal, Anna; Mi, Xiao; Talanov, Artem V.; Reppy, John D.

    2016-06-01

    In 2004, Kim and Chan (KC) reported a decrease in the period of torsional oscillators (TO) containing samples of solid 4He, as the temperature was lowered below 0.2 K [Kim E, Chan MHW (2004) Science 305(5692):1941–1944]. These unexpected results constituted the first experimental evidence that the long-predicted supersolid state of solid 4He may exist in nature. The KC results were quickly confirmed in a number of other laboratories and created great excitement in the low-temperature condensed-matter community. Since that time, however, it has become clear that the period shifts seen in the early experiments can in large part be explained by an increase in the shear modulus of the 4He solid identified by Day and Beamish [Day J, Beamish J (2007) Nature 450(7171):853–856]. Using multiple-frequency torsional oscillators, we can separate frequency-dependent period shifts arising from changes in the elastic properties of the solid 4He from possible supersolid signals, which are expected to be independent of frequency. We find in our measurements that as the temperature is lowered below 0.2 K, a clear frequency-dependent contribution to the period shift arising from changes in the 4He elastic properties is always present. For all of the cells reported in this paper, however, there is always an additional small frequency-independent contribution to the total period shift, such as would be expected in the case of a transition to a supersolid state.

  8. Search for supersolidity in solid 4He using multiple-mode torsional oscillators

    PubMed Central

    Eyal, Anna; Mi, Xiao; Talanov, Artem V.; Reppy, John D.

    2016-01-01

    In 2004, Kim and Chan (KC) reported a decrease in the period of torsional oscillators (TO) containing samples of solid 4He, as the temperature was lowered below 0.2 K [Kim E, Chan MHW (2004) Science 305(5692):1941–1944]. These unexpected results constituted the first experimental evidence that the long-predicted supersolid state of solid 4He may exist in nature. The KC results were quickly confirmed in a number of other laboratories and created great excitement in the low-temperature condensed-matter community. Since that time, however, it has become clear that the period shifts seen in the early experiments can in large part be explained by an increase in the shear modulus of the 4He solid identified by Day and Beamish [Day J, Beamish J (2007) Nature 450(7171):853–856]. Using multiple-frequency torsional oscillators, we can separate frequency-dependent period shifts arising from changes in the elastic properties of the solid 4He from possible supersolid signals, which are expected to be independent of frequency. We find in our measurements that as the temperature is lowered below 0.2 K, a clear frequency-dependent contribution to the period shift arising from changes in the 4He elastic properties is always present. For all of the cells reported in this paper, however, there is always an additional small frequency-independent contribution to the total period shift, such as would be expected in the case of a transition to a supersolid state. PMID:27222579

  9. Testing the U-Th/4He dating method on carbonates I. Helium diffusion

    NASA Astrophysics Data System (ADS)

    Pinti, D. L.; Ghaleb, B. G.; Sano, Y.; Blanchette, S.; Mathouchanh, E.; Takahata, N.

    2012-12-01

    Corals and other carbonates, such as speleothems, are important climatic-change proxies which need to be precisely dated for paleoclimatic reconstructions. Yet, U-Th disequilibrium method is applicable up to ca. 500 ka old carbonates. Calcite is difficult to date precisely by U-Pb method because of the low U amounts often found and difficulties in correcting for the common lead. Radiogenic 4He produced by decay of 238U and 235U incorporated into carbonates is a potential chronometer of Quaternary, and possibly Tertiary, corals and speleothems. However, several limitations exist for this method, related to the few data on the He diffusion [1] and on the alpha recoil effect in carbonate minerals. We decided to measure 4He by step heating in carbonate samples dated previously by U-Th disequilibrium: a coral (Scleractinia) from Cape Verde dated at 125 ka; a stalagmite from Patagonia dated at 128 ka; and two hydrothermal travertines from the Ziz Valley in Morocco with ages ≥ 500 ka. A one cm3 of each sample was cut by saw, crushed, washed and sieved to 80-100μm and 100-125μm fractions. Crushed samples (0.5 to 1 gram) were loaded in a vacuum crucible and 4He extracted by step heating. Previous step heating experiments on a sub-Arctic flowstone suggested that 4He is mainly released between 400 and 600°C [2]. However, the first coral sample heated at 100°C steps, showed a release pattern profile with 4He mainly released between 200 and 400°C. Measured 4He amount of 2.05 x 10-8 (±0.03% 1σ) ccSTP/g and U content of 2.7 ppm yield a U-4He age of 62.5 ka, lower than that obtained by U-Th disequilibrium. Data were not precise enough to calculate diffusion parameters using the Arrhenius diagram. The second step-heating pyrolysis of the coral using 50°C-steps indicated that all 4He is released between 250 and 350°C. The measured 4He amount was 2.27 x 10-8 (±0.04% 1σ) ccSTP/g, yielding an age of 83 ka, again lower compared to that obtained by U-Th disequilibrium. The

  10. Alpha Cluster States and Condensation in ^{16}O

    NASA Astrophysics Data System (ADS)

    Funaki, Y.; Yamada, T.; Horiuchi, H.; Röpke, G.; Schuck, P.; Tohsaki, A.

    Low density states near the 4α breakup threshold in ^{16}O is discussed in terms of the α-particle condensation. Calculations are performed with OCM (Orthogonality Condition Model) and GEM (Gauss Expansion Method). The 0_6^+ state in ^{16}O is shown to have a character of the 4α condensate, as an analogue to the Hoyle state in ^{12}C. The decay property of the s tate and the α + Hoyle-like rotatinal states are also investigated.

  11. Airy structure in 16O+14C nuclear rainbow scattering

    NASA Astrophysics Data System (ADS)

    Ohkubo, S.; Hirabayashi, Y.

    2015-08-01

    The Airy structure in 16 O +14 C rainbow scattering is studied with an extended double-folding (EDF) model that describes all the diagonal and off-diagonal coupling potentials derived from the microscopic realistic wave functions for 16 O by using a density-dependent nucleon-nucleon force. The experimental angular distributions at EL=132 , 281, and 382.2 MeV are well reproduced by the calculations. By studying the energy evolution of the Airy structure, the Airy minimum around θ =76∘ in the angular distribution at EL=132 MeV is assigned as the second-order Airy minimum A 2 in contrast to the recent literature which assigns it as the third order A 3 . The Airy minima in the 90∘ excitation function is investigated in comparison with well-known 16 O +16 O and 12 C +12 C systems. Evolution of the Airy structure into the molecular resonances with the 16 O +14 C cluster structure in the low-energy region around Ec .m .=30 MeV is discussed. It is predicted theoretically for the first time for a non-4 N 16O +14 C system that Airy elephants in the 90∘ excitation function are present.

  12. Temperature and pressure dependence of viscosity of quantum liquid 4He according to significant structure theory

    PubMed Central

    Ryoo, Ryong; John, Mu Shik; Eyring, Henry

    1980-01-01

    Both solid-like and gas-like flow structures are considered in the calculation of viscosity of liquid 4He using the significant structure theory of liquids. The predominance of quantum mechanical zero-point motion over that arising from thermal excitation is taken into account for the solid-like motion of molecules. The viscosity of liquid 4He under its own vapor pressure calculated over its whole temperature range is in reasonably good agreement with experimental data. The pressure dependence of viscosity also was obtained. The calculation does not yield good results at high densities where the free jumping of molecules into the nearest neighboring vacancies through the kinetic zero-point motion is no longer plausible. PMID:16592856

  13. Apatite 4He/3He and (U-Th)/He evidence for an ancient Grand Canyon.

    PubMed

    Flowers, R M; Farley, K A

    2012-12-21

    The Grand Canyon is one of the most dramatic features on Earth, yet when and why it was carved have been controversial topics for more than 150 years. Here, we present apatite (4)He/(3)He thermochronometry data from the Grand Canyon basement that tightly constrain the near-surface cooling history associated with canyon incision. (4)He/(3)He spectra for eastern Grand Canyon apatites of differing He date, radiation damage, and U-Th zonation yield a self-consistent cooling history that substantially validates the He diffusion kinetic model applied here. Similar data for the western Grand Canyon provide evidence that it was excavated to within a few hundred meters of modern depths by ~70 million years ago (Ma), in contrast to the conventional model in which the entire canyon was carved since 5 to 6 Ma.

  14. Sonofusion: Heat and ^4He Created by Cavitationally Induced Loading of Metal Foils

    NASA Astrophysics Data System (ADS)

    Stringham, Roger

    2003-03-01

    Helium four was produced in a vacuum tight system and measured by mass spectrometry with no measurable accompanying radiation. This fusion product from a piezo driven, acoustic reactor forces deuterons into a metallic foil. We believe the reaction is the result of the adiabatic collapse of transient bubbles in D_2O. The collapse process forms high-density plasma jets that are further z-pinched and then implanted into the foil lattices where the DD fusion takes place. With no evidence of long range radiation, the mc^2 energy was converted to heat. The reactor gases were analyzed at levels as high as 500 ppm of ^4He, which is 100 times that found in air. The SEM, Scanning Electron Microscope, photos of target foil surfaces show evidence of violent activity identified as ejecta sites varying in size from 100 to 10000 nm in diameter. The ^4He, radiation, excess heat, and SEM measurements support the DD fusion explanation.

  15. WORM ALGORITHM PATH INTEGRAL MONTE CARLO APPLIED TO THE 3He-4He II SANDWICH SYSTEM

    NASA Astrophysics Data System (ADS)

    Al-Oqali, Amer; Sakhel, Asaad R.; Ghassib, Humam B.; Sakhel, Roger R.

    2012-12-01

    We present a numerical investigation of the thermal and structural properties of the 3He-4He sandwich system adsorbed on a graphite substrate using the worm algorithm path integral Monte Carlo (WAPIMC) method [M. Boninsegni, N. Prokof'ev and B. Svistunov, Phys. Rev. E74, 036701 (2006)]. For this purpose, we have modified a previously written WAPIMC code originally adapted for 4He on graphite, by including the second 3He-component. To describe the fermions, a temperature-dependent statistical potential has been used. This has proven very effective. The WAPIMC calculations have been conducted in the millikelvin temperature regime. However, because of the heavy computations involved, only 30, 40 and 50 mK have been considered for the time being. The pair correlations, Matsubara Green's function, structure factor, and density profiles have been explored at these temperatures.

  16. Superheat Limit of 4He and Its Quantum Deviation from Classical Behavior

    NASA Astrophysics Data System (ADS)

    Nishigaki, Kazu; Saji, Yoshiro

    1983-07-01

    The superheating of normal liquid 4He was investigated by means of continuous heating of liquid specimen in a small glass capillary over a temperature range 2.26 K to 4.88 K. The maximum superheating data obtained were compared with the prediction from the homogeneous nucleation theory and the data for various liquids in terms of the reduced coordinates. It is confirmed that the agreement between the homogeneous nucleation theory and experiment on 4He is satisfactory, and the scaled superheating depends parametrically on the quantum parameter \\varLambda*, i.e., the deviations of the data for quantum liquids from the classical behavior become pronounced as the parameter is increased.

  17. Apatite 4He/3He and (U-Th)/He evidence for an ancient Grand Canyon.

    PubMed

    Flowers, R M; Farley, K A

    2012-12-21

    The Grand Canyon is one of the most dramatic features on Earth, yet when and why it was carved have been controversial topics for more than 150 years. Here, we present apatite (4)He/(3)He thermochronometry data from the Grand Canyon basement that tightly constrain the near-surface cooling history associated with canyon incision. (4)He/(3)He spectra for eastern Grand Canyon apatites of differing He date, radiation damage, and U-Th zonation yield a self-consistent cooling history that substantially validates the He diffusion kinetic model applied here. Similar data for the western Grand Canyon provide evidence that it was excavated to within a few hundred meters of modern depths by ~70 million years ago (Ma), in contrast to the conventional model in which the entire canyon was carved since 5 to 6 Ma. PMID:23196906

  18. Competition between thermal fluctuations and disorder in the crystallization of 4He in aerogel.

    PubMed

    Nomura, Ryuji; Osawa, Aiko; Mimori, Tomohiro; Ueno, Ken-ichi; Kato, Haruko; Okuda, Yuichi

    2008-10-24

    The dynamical transition in the crystallization of 4He in aerogel has been investigated by direct visualization and dynamical phase diagrams have been determined. The crystal-superfluid interface in aerogel advances via creep at high temperatures and avalanches at low temperatures. The transition temperature is higher at a higher interface velocity and lower in higher porosity aerogels. The transition is due to competition between thermal fluctuations and disorder for the crystallization process. PMID:18999765

  19. Production of {sup 4}He and tritium from Be in the COBRA-1A2 irradiation

    SciTech Connect

    Greenwood, L.R.

    1998-03-01

    The production of {sup 4}He and tritium has been calculated for beryllium irradiated in the COBRA-1A2 experiment in the Experimental Breeder Reactor II. Reaction rates were based on adjusted neutron spectra determined from reactor dosimetry measurements at three different elevations in the region of the beryllium capsules. Equations are given so that gas production can be calculated for any specific capsule elevation.

  20. Anomalous 4He Observation with EPHIN on Board SOHO during 1996 and 1997

    NASA Astrophysics Data System (ADS)

    Gómez-Herrero, R.; Del Peral, L.; Rodríguez-Frías, D.; Sequeiros, J.; Gutiérrez, J.; Müller-Mellin, R.; Kunow, H.

    2003-07-01

    The analysis of the 4 He spectrum during solar quiet time periods has demonstrated that the main source is of anomalous origin. It has been determined that this anomalous component reached similar levels to the observed ones during the 1976 solar minimum, revealing the importance of the solar polarity in the particle transport inside the heliosphere. Acceleration conditions of anomalous cosmic rays in the solar wind termination shock have been obtained.

  1. Primary populations of metastable antiprotonic (4)He and (3)He atoms.

    PubMed

    Hori, M; Eades, J; Hayano, R S; Ishikawa, T; Sakaguchi, J; Tasaki, T; Widmann, E; Yamaguchi, H; Torii, H A; Juhász, B; Horváth, D; Yamazaki, T

    2002-08-26

    Initial distributions of metastable antiprotonic (4)He and (3)He atoms over principal (n) and angular momentum (l) quantum numbers have been deduced using laser spectroscopy experiments. The regions n = 37-40 and n = 35-38 in the two atoms account for almost all of the observed fractions [(3.0 +/- 0.1)% and (2.4 +/- 0.1)%] of antiprotons captured into metastable states. PMID:12190401

  2. A new method for determining the 3He/4He ratio in the local interstellar medium

    NASA Astrophysics Data System (ADS)

    Lemoine, M.; Vidal-Madjar, A.; Ferlet, R.

    1993-06-01

    We propose here an original method for estimating the 3He/4 Heratio in the local diffuse interstellar medium at a low cost from an observational point of view. The main idea is to measure the shift in radial velocity of the 4He λ537Å and λ584Å lines due to the presence of 3He in the red wing of these lines, and to compare the observed shift to the shifts obtained through numerical simulations for different 3He/4He ratios. We performed such simulations in order to reveal the efficiency of this method, using typical astrophysical conditions and instrumental parameters corresponding to the Lyman-FUSE mission. We find that this method should yield the 3He/4He ratio with a 1 σ uncertainty ˜50% at a spectral resolving power R=30 000 and a signal-to-noise ratio S/N=50. This method thus appears more adapted to a forehand estimation of the interstellar 3He/4He ratio than the standard profile fitting method, which should yield a 1 σ uncertainty of 10% at R=30 000 and S/N ≃ 290 (Hurwitz & Bowyer, t985). Finally, our method should be able to settle the evolutionary status of 3He if 3He has been significantly enhanced or depleted in the last 4.6 Gyr. Combined with the measurement of the deuterium abundance on the same line of sight (already programmed on HST), this might yield very important constraint on Big-Bang nucleosynthesis consistency.

  3. Electronically tunable fiber laser for optical pumping of {sup 3}He and {sup 4}He

    SciTech Connect

    Stephens, E.F.; Patrick, H.; Gilbert, S.L.

    1996-03-01

    We present in this paper a low threshold, highly stable, integrated fiber laser cavity that uses an electronically tunable internal Bragg grating. The fiber laser produced over 5 mW with a spectral width of about 5 GHz at 1083 nm. The laser was used to achieve 30{percent} polarization of the 2{sup 3}{ital S}{sub 1} metastable states of {sup 4}He in a weak rf discharge cell. {copyright} {ital 1996 American Institute of Physics.}

  4. Wave Turbulence in Superfluid {sup 4}He: Energy Cascades and Rogue Waves in the Laboratory

    SciTech Connect

    Efimov, V. B.; Ganshin, A. N.; McClintock, P. V. E.; Kolmakov, G. V.; Mezhov-Deglin, L. P.

    2008-11-13

    Recent work on second sound acoustic turbulence in superfluid {sup 4}He is reviewed. Observations of forward and inverse energy cascades are described. The onset of the inverse cascade occurs above a critical driving energy and it is accompanied by giant waves that constitute an acoustic analogue of the rogue waves that occasionally appear on the surface of the ocean. The theory of the phenomenon is outlined and shown to be in good agreement with the experiments.

  5. Observation of a Dislocation-Related Interfacial Friction Mechanism in Mobile Solid 4He

    NASA Astrophysics Data System (ADS)

    Eyal, Anna; Livne, Ethan; Polturak, Emil

    2016-04-01

    We report a study of the temperature and stress dependence of the friction associated with a relative motion of crystallites of solid 4He in contact with each other. A situation where such motion exists emerges spontaneously during a disordering of a single crystal contained inside an annular sample space of a torsional oscillator (TO). Under the torque applied by the oscillating walls of the TO these crystallites move relative to each other, generating measurable dissipation at their interface. We studied this friction between 0.5 and 1.8 K in solid samples grown from commercially pure 4He and from a 100 ppm 3He-4He mixture. The data were analyzed by modeling the TO as a driven harmonic oscillator. In this model, an analysis of the resonant frequency and amplitude of the TO yields the temperature dependence of the friction coefficient. By fitting the data to specific forms, we found that over our temperature range, the dominant friction mechanism associated with the interfacial motion of the crystallites results from climb of individual dislocations. The characteristic energy scale associated with this friction can be 3 or 6 K, depending on the sample. The motion of the solid in the presence of such friction can perhaps be described as the low limit of "slip-stick" motion.

  6. Phase equilibrium in a polarized saturated {sup 3}He-{sup 4}He mixture

    SciTech Connect

    Rodrigues, A.; Vermeulen, G.

    1997-07-01

    We present experimental results on the phase equilibrium of a saturated {sup 3}He-{sup 4}He mixture, which has been cooled to a temperature of 10-15 mK and polarized in a {sup 4}He circulating dilution refrigerator to a stationary polarization of 15 %, 7 times higher than the equilibrium polarization in the external field of 7 T. The pressure dependence of the polarization enhancement in the refrigerator shows that the molar susceptibilities of the concentrated and dilute phase of a saturated {sup 3}He-{sup 4}He mixture are equal at p = 2.60 {+-} 0.04 bar. This result affects the Fermi liquid parameters of the dilute phase. The osmotic pressure in the dilute phase has been measured as a function of the polarization of the coexisting concentrated phase up to 15 %. We find that the osmotic pressure at low polarization ( < 7 % ) agrees well with thermodynamics using the new Fermi liquid parameters of the dilute phase.

  7. New solar axion search using the CERN Axion Solar Telescope with 4He filling

    NASA Astrophysics Data System (ADS)

    Arik, M.; Aune, S.; Barth, K.; Belov, A.; Bräuninger, H.; Bremer, J.; Burwitz, V.; Cantatore, G.; Carmona, J. M.; Cetin, S. A.; Collar, J. I.; Da Riva, E.; Dafni, T.; Davenport, M.; Dermenev, A.; Eleftheriadis, C.; Elias, N.; Fanourakis, G.; Ferrer-Ribas, E.; Galán, J.; García, J. A.; Gardikiotis, A.; Garza, J. G.; Gazis, E. N.; Geralis, T.; Georgiopoulou, E.; Giomataris, I.; Gninenko, S.; Gómez Marzoa, M.; Hasinoff, M. D.; Hoffmann, D. H. H.; Iguaz, F. J.; Irastorza, I. G.; Jacoby, J.; Jakovčić, K.; Karuza, M.; Kavuk, M.; Krčmar, M.; Kuster, M.; Lakić, B.; Laurent, J. M.; Liolios, A.; Ljubičić, A.; Luzón, G.; Neff, S.; Niinikoski, T.; Nordt, A.; Ortega, I.; Papaevangelou, T.; Pivovaroff, M. J.; Raffelt, G.; Rodríguez, A.; Rosu, M.; Ruz, J.; Savvidis, I.; Shilon, I.; Solanki, S. K.; Stewart, L.; Tomás, A.; Vafeiadis, T.; Villar, J.; Vogel, J. K.; Yildiz, S. C.; Zioutas, K.; CAST Collaboration

    2015-07-01

    The CERN Axion Solar Telescope (CAST) searches for a →γ conversion in the 9 T magnetic field of a refurbished LHC test magnet that can be directed toward the Sun. Two parallel magnet bores can be filled with helium of adjustable pressure to match the x-ray refractive mass mγ to the axion search mass ma. After the vacuum phase (2003-2004), which is optimal for ma≲0.02 eV , we used 4He in 2005-2007 to cover the mass range of 0.02-0.39 eV and 3He in 2009-2011 to scan from 0.39 to 1.17 eV. After improving the detectors and shielding, we returned to 4He in 2012 to investigate a narrow ma range around 0.2 eV ("candidate setting" of our earlier search) and 0.39-0.42 eV, the upper axion mass range reachable with 4He, to "cross the axion line" for the KSVZ model. We have improved the limit on the axion-photon coupling to ga γ<1.47 ×10-10 GeV-1 (95% C.L.), depending on the pressure settings. Since 2013, we have returned to the vacuum and aim for a significant increase in sensitivity.

  8. Active Inspection of Nuclear Materials Using {sup 4}He Scintillation Detectors

    SciTech Connect

    Davatz, G.; Howard, A.; Chandra, R.; Gendotti, U.

    2011-12-13

    The detection of fissionable materials by neutron and high-energy photon active interrogation methods is explored using {sup 4}He scintillation detectors to search for prompt and delayed neutron signature. The low electron density of {sup 4}He in addition to its pulse shape discrimination capability allows strong rejection of gamma radiation. For the detection of the prompt neutron signatures, this capability is important as the signal produced by induced fission is accompanied by intense gamma radiation. The nanosecond time resolution of {sup 4}He scintillation detectors can be used for time-of-flight measurements aimed at determining the energy of the emitted neutrons. For delayed neutron detection, the insensitivity to the low energy neutrons present from non-signal reactions is inherent. Unlike detectors requiring a moderator, this technology can easily be collimated to reduce sensitivity to neutrons from outside the field of interest. The performance of the detectors for these applications is studied using GEANT4 computer modeling, based on measured detector parameters. A comparison is made with technologies typically used for these applications, i.e. heavily shielded organic scintillators for prompt neutron detection and Cd-lined {sup 3}He neutron detectors for the detection of delayed neutrons.

  9. Capillary Condensation of Liquid 4He in Aerogel on Cooling Through {lambda} Point

    SciTech Connect

    Miyashita, W.; Yoneyama, K.; Kato, H.; Nomura, R.; Okuda, Y.

    2006-09-07

    Capillary condensation of liquid 4He in silica aerogel with a 90% porosity was investigated visually. The initial condition of the experiment was such that liquid 4He was present in the sample cell but not in the aerogel. This situation was realized by introducing the liquid into the cell at a fast rate to avoid liquefaction in the aerogel. The free surface of the liquid rose up in the cell with filling and eventually reached the bottom of the aerogel. Then, the aerogel absorbed the liquid by capillary condensation. The height of the liquid in the aerogel rose with time t roughly as t1/2 in the normal fluid phase. This behavior was consistent with the Washburn model. When the system was cooled through the {lambda} point during the condensation, the liquid height started to rise faster in the superfluid phase with a constant velocity of about 0.3 mm/sec. The dynamics of capillary condensation was strongly dependent on whether the liquid 4He was in the normal or the superfluid phase.

  10. On the Evolution of the Light Elements. I. D, 3He, and 4He

    NASA Astrophysics Data System (ADS)

    Fields, Brian D.

    1996-01-01

    The light elements D, 3He, 4He, and 7Li are produced in big bang nucleosynthesis and undergo changes in their abundances due to Galactic processing. Since one may observe most of these elements only in contemporary environments, knowledge of the intervening evolution is necessary for determining the observational constraints on primordial nucleosynthesis Chemical and stellar evolution model dependences in light element evolution are systematically investigated via a comparison of 1460 possible chemical evolution scenarios and a comparison of stellar nucleosynthesis yields, all of which have been selected to fit solar neighborhood C, N, 0, and Fe abundances as well as the observed local gas density and gas mass fraction. The light element evolution and solar system yields in these models are found to span a wide range, explicitly demonstrating the model dependence. The range of model dependence for D, 3He, and 4He solar abundances is calculated, and its sensitivity to the heavy element constraints is noted. The chemical evolution contribution to the uncertainty in the observed primordial light element abundances is estimated, and the effects of this uncertainty on big bang nucleosynthesis results are discussed. The predictions for the light elements are found to be correlated; the extent and physical origin of these correlations is discussed. D and 3He evolution is found to have significant model dependence; however, the dominant factor determining their solar and interstellar abundances is their primordial abundance. In addition, 3He is found to be very sensitive to the details of processing in low-mass stars. 4He yields are shown to be very model dependent. In particular, both the introduction of mass loss and the possibly very high 4He stellar yields in the poorly understood mass range of ˜8-12Msun can lead to large enhancement of 4He production and can lead to large slopes of ΔY/ΔN and ΔY/ΔO. It is found that the inclusion of secondary nitrogen leads to

  11. Alpha decay widths of excited states of 16O

    NASA Astrophysics Data System (ADS)

    Haigh, P. J.; Freer, M.; Ashwood, N. I.; Bloxham, T.; Curtis, N.; Bohlen, H. G.; Dorsch, T.; Kokalova, Tz; Wheldon, C.; Catford, W. N.; Patterson, N. P.; Thomas, J. S.

    2010-03-01

    The 12C(13C, 9Be)16O reaction has been used to populate excited states in 16O. The 9Be nuclei were detected in a magnetic spectrometer and the 12C decay product of the recoiling excited 16O nucleus was detected in an array of silicon strip detectors. The large angular coverage of the strip detector array allowed the α-decay widths of the 14.66 MeV, 5-, and 16.275 MeV, 6+, states to be determined with good accuracy. The present results, together with earlier measurements, allow precise values for the branching ratios to be calculated: Ex(16O) = 14.66 MeV, Jπ = 5-, Γα0/Γ = 0.951 ± 0.049 and Γα1/Γ < 0.05; Ex(16O) = 16.275 MeV, Jπ = 6+, Γα0/Γ = 0.982 ± 0.048 and Γα1/Γ < 0.02.

  12. Precision prediction for the big-bang abundance of primordial 4He

    NASA Astrophysics Data System (ADS)

    Lopez, Robert E.; Turner, Michael S.

    1999-05-01

    Within the standard models of particle physics and cosmology we have calculated the big-bang prediction for the primordial abundance of 4He to a theoretical uncertainty of less than 0.1% (δYP<+/-0.0002), improving the current theoretical precision by a factor of 10. At this accuracy the uncertainty in the abundance is dominated by the experimental uncertainty in the neutron mean lifetime, τn=885.4+/-2.0 sec. The following physical effects were included in the calculation: the zero and finite-temperature radiative, Coulomb and finite-nucleon-mass corrections to the weak rates; order-α quantum-electrodynamic correction to the plasma density, electron mass, and neutrino temperature; and incomplete neutrino decoupling. New results for the finite-temperature radiative correction and the QED plasma correction were used. In addition, we wrote a new and independent nucleosynthesis code designed to control numerical errors to be less than 0.1% . Our predictions for the 4He abundance are presented in the form of an accurate fitting formula. Summarizing our work in one number, YP(η=5×10-10)=0.2462+/-0.0004 (expt) +/-<0.0002 (theory). Further, the baryon density inferred from the Burles-Tytler determination of the primordial D abundance, ΩBh2=0.019+/-0.001, leads to the prediction YP=0.2464+/-0.0005 (D/H) +/-<0.0002 (theory) +/-0.0005 (expt). This ``prediction'' and an accurate measurement of the primeval 4He abundance will allow an important consistency test of primordial nucleosynthesis.

  13. Heat Capacity of Superfluid (sup 4)He in the Presence of a Heat Current Near T

    NASA Technical Reports Server (NTRS)

    Chui, Talso C. P.; Goodstein, David L.; Harter, Alexa W.; Mukhopadhyay, Ranjan

    1996-01-01

    The thermodynamic theory of superfluid helium in the presence of a heat current is presented. We show that there is a thermodynamic relation between the heat capacity and the expression ps(W), which describes the depression of the superfluid density with the counterflow velocity W. Using this relation we show that the heat capacity of superfluid super4He in the presence of a heat current diverges at a depressed lambda transition temperature, suggesting the possibility of a new second order phase transition where the superfluid wave function is not the order parameter.

  14. Measurements of Vortex Line Density Generated by a Quartz Tuning Fork in Superfluid 4He

    NASA Astrophysics Data System (ADS)

    Jackson, M. J.; Kolosov, O.; Schmoranzer, D.; Skrbek, L.; Tsepelin, V.; Woods, A. J.

    2016-05-01

    We present proof-of-concept measurements of the vortex line density generated by a quartz tuning fork resonator probed by the attenuation of second sound in superfluid ^4He at 1.6 K. The force-velocity response of a quartz tuning fork operating at a frequency of 31 kHz exhibited the onset of extra damping at a velocity of 0.5 ms^{-1}. Attenuation of the 5th resonant mode of second sound was observed at the same velocity, indicating the production of vortex lines. Our measurements demonstrate that an increase of the drag coefficient corresponds to the development of quantum turbulence.

  15. Torsional oscillator and synchrotron x-ray experiments on solid {sup 4}He in aerogel.

    SciTech Connect

    Mulders, N.; West, J. T.; Chan, M. H. W.; Kodituwakku, C. N.; Burns, C. A.; Lurio, L. B.; Univ. of Delaware; Pennsylvania State Univ.; Western Michigan Univ.; Northern Illinois Univ.

    2008-01-01

    X-ray diffraction experiments show that solid {sup 4}He grown in aerogel is highly polycrystalline, with an hcp crystal structure (as in bulk) and a crystallite size of approximately 100 nm. In contrast to the expectation that the highly disordered solid will have a large supersolid fraction, torsional oscillator measurements show a behavior that is strikingly similar to high purity crystals grown from the superfluid phase. The low temperature supersolid fraction is only {approx}3 x 10{sup -4}, and the onset temperature is {approx}100 mK.

  16. Quantum Tunneling of ^3He in Solid ^4He: A New Analysis

    NASA Astrophysics Data System (ADS)

    Huan, C.; Kim, S. S.; Candela, D.; Sullivan, N. S.

    2016-11-01

    We discuss the analysis of the experimental values of the nuclear spin-lattice and spin-spin relaxation times for the tunneling of ^3He as isotopic impurities in solid ^4He. These two relaxation times cannot be described quantitatively using a unique correlation time although it is often presented as such in the literature. In this paper, we discuss how to distinguish the high-frequency portion of the spectral densities that determine the spin-lattice relaxation rates from the low-frequency components which determine the spin-spin relaxation rates.

  17. 4He Implantation in Natural Diamond: Implications for Apatite (U-Th)/He Thermochronometry

    NASA Astrophysics Data System (ADS)

    Phillips, D.; Kohn, B. P.; Gleadow, A. J.; Harris, J. W.

    2007-12-01

    Current apatite (U-Th)/He thermochronometry protocols correct for ejection of α-particles from grain margins. However, the potential for implantation of 4He into apatite grains, from primary or secondary actinide minerals, has received more limited attention. Evidence for significant natural α-fluxes in the near- surface environment is provided by surface feature and He abundance studies on diamond. Intense α- damage induces a green colour centre in diamond, enabling visual assessment of natural α-implantation doses. Diamonds with transparent green coats and/or green spots occur in most primary and detrital diamond deposits worldwide, indicating that α-implantation rates into upper crustal minerals may be more significant than previously envisaged. Experiments on transparent green-coated natural diamonds reveal implanted αHe concentrations up to 0.015 cc/g, attributed to secondary uranium phases deposited by circulating groundwater (Shelkov et al., 1998). Implantation of similar α-dosages into apatite grains would increase (U-Th)/He ages by up to several hundred percent, dependent on α-dose rate, grain dimensions and actinide content. Investigation of actinide-rich granites in Australia has revealed the common juxtaposition of apatite and actinide phases such as monazite and zircon. In addition, secondary actinide-bearing phases (e.g. uraninite) are observed along joints, fractures, miarolitic cavities and weathering fronts, thus providing additional α-sources. These results demonstrate that (U-Th)/He thermochronometry analyses of apatite, particularly from actinide-rich, weathered granites and sediments, need to evaluate the potential for 4He implantation in the near-surface environment. Insight into the extent of this problem may be achievable through multiple analyses of single grains, in situ laser probe analyses, 4He/3He step-heating experiments, abrasion of grains and/or complementary apatite fission track analyses. Reference: Shelkov, D

  18. Communication: Nucleation of quantized vortex rings in {sup 4}He nanodroplets

    SciTech Connect

    Mateo, David; Leal, Antonio; Barranco, Manuel; Pi, Martí; Hernando, Alberto; Cargnoni, Fausto; Mella, Massimo; Zhang, Xiaohang; Drabbels, Marcel

    2014-04-07

    Whereas most of the phenomena associated with superfluidity have been observed in finite-size helium systems, the nucleation of quantized vortices has proven elusive. Here we show using time-dependent density functional simulations that the solvation of a Ba{sup +} ion created by photoionization of neutral Ba at the surface of a {sup 4}He nanodroplet leads to the nucleation of a quantized ring vortex. The vortex is nucleated on a 10 ps timescale at the equator of a solid-like solvation structure that forms around the Ba{sup +} ion. The process is expected to be quite general and very efficient under standard experimental conditions.

  19. Measurements of Superfluid 4He Flow Through Sub-15 nm Aperture Arrays

    SciTech Connect

    Hoffmann, J. A.; Hunt, B.; Wang, M.; Davis, J. C.; Black, C. T.

    2006-09-07

    We have constructed an experiment designed to study Josephson phenomena in 4He. Motivated by reports and our ideas for novel silicon nanofabrication techniques, we designed the experiment to study the possibility of a transition from stochastic to coherent phase slippage. Here we briefly describe the nanofabrication of sub-15 nm aperture arrays and show preliminary data. For temperatures below 2 K, these data show temperature dependence of the superfluid critical velocity through the weak link which is characteristic of phase-slip limited flow.

  20. Spatially Extended Avalanches in a Hysteretic Capillary Condensation System: Superfluid {sup {bold 4}}He in Nuclepore

    SciTech Connect

    Lilly, M.P.; Wootters, A.H.; Hallock, R.B.

    1996-11-01

    Capacitive studies of hysteretic capillary condensation of superfluid {sup 4}He in Nuclepore have shown that the initial draining of the pores occurs over a small range of the chemical potential with avalanches present as groups of pores drain. In the work reported here, the avalanches in this system are shown to be nonlocal events which involve pores distributed at low density across the entire sample. The nonlocal avalanche behavior is shown to be enabled by the presence of a superfluid film connection among the pores. {copyright} {ital 1996 The American Physical Society.}

  1. Formation of a Mesa Shaped Phonon Pulse in Superfluid 4He

    NASA Astrophysics Data System (ADS)

    Adamenko, I. N.; Nemchenko, K. E.; Slipko, V. A.

    2010-05-01

    We present a theory for the formation of a mesa shaped phonon pulse in superfluid 4He. Starting from the hydrodynamic equations of superfluid helium, we obtain the system of equations which describe the evolution of strongly anisotropic phonon systems. Such systems can be created experimentally. The solution of the equations are simple waves, which correspond to second sound in the moving phonon pulse. Using these exact solutions, we describe the expansion of phonon pulses in superfluid helium at zero temperature. This theory gives an explanation for the mesa shape observed in the measured phonon angular distributions. Almost all dependencies of the mesa shape on the system parameters can be qualitatively understood.

  2. Velocity distributions of tracer particles in thermal counterflow in superfluid 4He

    NASA Astrophysics Data System (ADS)

    Mineda, Yoshikazu; Tsubota, Makoto; Sergeev, Yuri A.; Barenghi, Carlo F.; Vinen, W. F.

    2013-05-01

    Quantum turbulence accompanying thermal counterflow in superfluid 4He was recently visualized by the Maryland group, using micrometer-sized tracer particles of solid hydrogen [Paoletti, Fiorito, Sreenivasan, and Lathrop, J. Phys. Soc. Jpn.10.1143/JPSJ.77.111007 77, 111007 (2008)]. In order to understand the observations, we formulate the coupled dynamics of fine particles and quantized vortices, in the presence of a relative motion of the normal and superfluid components. Numerical simulations based on this formulation are shown to agree reasonably well with experimental observations of the velocity distributions of the tracer particles in thermal counterflow.

  3. Simultaneous measurements of the torsional oscillator anomaly and thermal conductivity in solid 4He.

    PubMed

    Zmeev, D E; Golov, A I

    2011-08-01

    In these torsional oscillator experiments, the samples of solid (4)He were characterized by measuring their thermal conductivity. Polycrystalline samples of helium of either high isotopic purity or natural concentration of (3)He were grown in an annular container by the blocked-capillary method and investigated before and after annealing. No correlation has been found between the magnitude of the low-temperature shift of the torsional oscillator frequency and the amount of crystalline defects as measured by the thermal conductivity. In samples with the natural (3)He concentration, a substantial excess thermal conductivity over the usual T(3) dependence was observed below 120 mK.

  4. Dynamics of the BCC-HCP transition of solid 4He

    NASA Astrophysics Data System (ADS)

    Fujii, Hirosuke; Okumura, Yuji; Matsumoto, Koichi; Okuda, Yuichi

    2000-07-01

    We are optically studying the phase transition from BCC to HCP of solid 4He (1.43 K) at melting pressure to investigate how the crystal changes its structure when it is in equilibrium with superfluid. When the temperature was changed slowly through the transition, new phase seeds were nucleated somewhere and those seeds grew in the superfluid phase. The interesting point is that growth of the new seeds is more favorable than the direct solid-solid Martensitic transition. Whereas at the transition of 1.78 K where the solid is in equilibrium with the normal fluid, the transition occurred as an ordinary Martensitic transition.

  5. Crossover from hydrodynamic to acoustic drag on quartz tuning forks in normal and superfluid 4He

    NASA Astrophysics Data System (ADS)

    Bradley, D. I.; Človečko, M.; Fisher, S. N.; Garg, D.; Guise, E.; Haley, R. P.; Kolosov, O.; Pickett, G. R.; Tsepelin, V.; Schmoranzer, D.; Skrbek, L.

    2012-01-01

    We present measurements of the drag forces on quartz tuning forks oscillating at low velocities in normal and superfluid 4He. We have investigated the dissipative drag over a wide range of frequencies, from 6.5 to 600 kHz, by using arrays of forks with varying prong lengths and by exciting the forks in their fundamental and first overtone modes. At low frequencies the behavior is dominated by laminar hydrodynamic drag, governed by the fluid viscosity. At higher frequencies acoustic drag is dominant and is described well by a three-dimensional model of sound emission.

  6. Torsional oscillator experiment on superfluid 4He confined in a porous alumina nanopore array

    NASA Astrophysics Data System (ADS)

    Murakawa, S.; Higashino, R.; Yoshimura, K.; Chikazawa, Y.; Tanaka, T.; Kuriyama, K.; Honda, K.; Shibayama, Y.; Shirahama, K.

    2012-12-01

    We studied superfluidity of liquid 4He confined in an array of well-characterized straight nanopores of porous alumina (PA). The PA plate sample of 45 nm pore size is set in an annular flow channel and the superflow is detected by torsional oscillator (TO) technique. Superfluid transition Tc in the nanopores is suppressed by 3.5 mK from the bulk λ point. Tc is consistent with the temperature at which the healing length is equal to the pore radius. We have observed many anti-crossing anomalies in the TO frequency associated with dissipation peaks, which are attributed to the coupling to second sound resonances.

  7. 16O + 16O molecular structures of positive- and negative-parity superdeformed bands in 34S

    NASA Astrophysics Data System (ADS)

    Taniguchi, Yasutaka

    2016-05-01

    The structures of excited states in 34S are investigated using the antisymmetrized molecular dynamics and generator coordinate method(GCM). The GCM basis wave functions are calculated via energy variation with a constraint on the quadrupole deformation parameter β. By applying the GCM after parity and angular momentum projections, the coexistence of two positive- and one negative-parity super de formed(SD) bands are predicted, and low-lying states and other deformed bands are obtained. The SD bands have structures of 16O + 16O + two valence neutrons in molecular orbitals around the two 16O cores in a cluster picture. The configurations of the two valence neutrons are δ2 and π2 for the positive-parity SD bands and π1δ1 for the negative parity SD band.

  8. Spin-polarized hydrogen adsorbed on the surface of superfluid {sup 4}He

    SciTech Connect

    Marín, J. M.; Boronat, J.; Markić, L. Vranješ

    2013-12-14

    The experimental realization of a thin layer of spin-polarized hydrogen H↓ adsorbed on top of the surface of superfluid {sup 4}He provides one of the best examples of a stable, nearly two-dimensional (2D) quantum Bose gas. We report a theoretical study of this system using quantum Monte Carlo methods in the limit of zero temperature. Using the full Hamiltonian of the system, composed of a superfluid {sup 4}He slab and the adsorbed H↓ layer, we calculate the main properties of its ground state using accurate models for the pair interatomic potentials. Comparing the results for the layer with the ones obtained for a strictly 2D setup, we analyze the departure from the 2D character when the density increases. Only when the coverage is rather small the use of a purely 2D model is justified. The condensate fraction of the layer is significantly larger than in 2D at the same surface density, being as large as 60% at the largest coverage studied.

  9. Bose condensate in superfluid sup 4 He and momentum distributions by deep inelastic scattering

    SciTech Connect

    Silver, R.N. ); Sokol, P.E. . Dept. of Physics)

    1989-01-01

    There are several reasons for the high interest in the recent experimental and theoretical progress in understanding deep inelastic neutron scattering from liquid {sup 4}He: it tests the fundamental London hypothesis of a connection between superfluidity and Bose condensation; it provides a quantitative test of ab-initio calculational methods for all systems with strong correlations which are the focus of current quantum many-body research; and it establishes the range of validity of deep inelastic scattering as a method for measuring momentum distributions. In this paper we introduce the concepts of impulse approximation in more detail, we describe recent progress in the theory for final state corrections to the impulse approximation, we present quantitative predictions for neutron scattering experiments, we compare with recent high energy pulsed neutron source experiments on liquid {sup 4}He by P. Sokol and colleagues as well as other attempts to extract the Bose condensate fraction from the neutron scattering data, and we discuss the implications of this progress for future momentum distribution experiments in other systems such as liquid {sup 3}He and quasi-elastic electron nucleus scattering. 42 refs., 23 figs.

  10. Depression of the Superfluid Transition Temperature in 4He by a Heat Flow

    NASA Astrophysics Data System (ADS)

    Yin, Liang; Lin, Peng; Qi, Xin

    2014-11-01

    The depression of the superfluid transition temperature Tλ in 4He by a heat flow Q is studied. A small sealed cell with a capillary is introduced and a stable and flat superfluid transition temperature plateau is easily obtained by controlling the temperature of the variable-temperature platform and the bottom chamber of the sealed cell. Owing to the depression effect of the superfluid transition temperature by the heat flow, the heat flow through the capillary is changed by the temperature control to obtain multiple temperature plateaus of different heat flows. The thermometer self-heating effect, the residual heat leak of the 4.2 K environment, the temperature difference on the He II liquid column, the Kapiza thermal resistance between the liquid helium and the copper surface of the sealed cell, the temperature gradient of the sealed cell, the static pressure of the He II liquid column and other factors have influence on the depression effect and the influence is analyzed in detail. Twenty experiments of the depression of the superfluid transition temperature in 4He by heat flow are made with four sealed cells in one year. The formula of the superfluid transition temperature pressured by the heat flow is Tλ (Q) = -0.00000103Q + 2.1769108, and covers the range 229 <= Q <= 6462 μW/cm2.

  11. Giant isochoric compressibility of solid 4He: The bistability of superclimbing dislocations

    NASA Astrophysics Data System (ADS)

    Kuklov, A. B.

    2015-10-01

    A significant accumulation of matter in solid 4He observed during a superflow event, dubbed the giant isochoric compressibility (or the syringe effect), is discussed within the model of dislocations with superfluid core. It is shown that solid 4He in contact with a superfluid reservoir can develop a bistability with respect to the syringe fraction, with the threshold for the bias by chemical potential determined by a typical free length of dislocations with superfluid core. The main implications of this effect are hysteresis and strongly nonlinear dynamical behavior leading to growth, proliferation, and possibly exiting from a crystal of superclimbing dislocations. Three major channels for such dynamics are identified: (i) injection and inflation of the prismatic loops from the boundary, (ii) Bardeen-Herring generation of the loops in the bulk, and (iii) helical instability of the screw dislocations. It is argued that the syringe instability may have already been observed in the experiments on the superflow through solid Helium-4. Several testable predictions for the time and the bias dependencies of the dynamics are suggested.

  12. Excitations in a thin liquid {sup 4}He film from inelastic neutron scattering

    SciTech Connect

    Clements, B.E. |; Godfrin, H.; Krotscheck, E. |; Lauter, H.J.; Leiderer, P.; Passiouk, V. |; Tymczak, C.J.

    1996-05-01

    We perform a thorough analysis of the experimental dynamic structure function measured by inelastic neutron scattering for a low-temperature ({ital T}=0.65 K) four-layer liquid {sup 4}He film. The results are interpreted in light of recent theoretical calculations of the (nonvortex) excitations in thin liquid Bose films. The experimental system consists of four outer liquid layers, adsorbed to two solid inner {sup 4}He layers, which are themselves adsorbed to a graphite substrate. Relatively intense surface (ripplon) and bulklike modes are observed. The analysis of the experimental data gives strong evidence for still other modes and supports the long-standing theoretical predictions of layerlike modes (layer phonons) associated with excitations propagating primarily within the liquid layers comprising the film. The results of the analysis are consistent with the occurrence of level crossings between modes, and the existence of a layer modes for which the theory predicts will propagate in the vicinity of the solid-liquid interface. The theory and experiment agree on the detailed nature of the ripplon; its dispersion at low momenta, its fall off in intensity at intermediate momenta, and the level crossings at high momentum. Similar to experiment, the theory yields an intense mode in the maxon-roton region which is intrepreted as the formation of the bulklike excitation. {copyright} {ital 1996 The American Physical Society.}

  13. Missing Lead and High 3He/4He in Ancient Sulfides Associated with Continental Crust Formation

    PubMed Central

    Huang, Shichun; Lee, Cin-Ty A.; Yin, Qing-Zhu

    2014-01-01

    Major terrestrial reservoirs have Pb isotopes more radiogenic than the bulk silicate Earth. This requires a missing unradiogenic Pb reservoir, which has been argued to reside in the lower continental crust or dissolved in the core. Chalcophile element studies indicate that continent formation requires the formation of sulfide-bearing mafic cumulates in arcs. Because Pb, but not U, partitions into sulfides, we show that continent formation must have simultaneously generated time-integrated unradiogenic Pb reservoirs composed of sulfide-bearing cumulates, now recycled back into the mantle or stored deep in the continental lithosphere. The generation of such cumulates could also lead to coupled He-Pb isotopic systematics because 4He is also produced during U-Th-Pb decay. Here, we show that He may be soluble in sulfide melts, such that sulfide-bearing cumulates would be enriched in both Pb and He relative to U and Th, “freezing” in He and Pb isotopes of the ambient mantle at the time of sulfide formation. This implies that ancient sulfide-bearing cumulates would be characterized by unradiogenic Pb and He isotopes (high-3He/4He). These primitive signatures are usually attributed to primordial, undifferentiated mantle, but in this case, they are the very imprint of mantle differentiation via continent formation. PMID:24937103

  14. Experiments on the rapid mechanical expansion of liquid 4He through its superfluid transition.

    PubMed

    Efimov, V B; Griffiths, O J; Hendry, P C; Kolmakov, G V; McClintock, P V E; Skrbek, L

    2006-11-01

    Phenomena following a rapid mechanical quench of liquid 4He from its normal to its superfluid phase are reported and discussed. The mechanical expansion apparatus is an improved version of that described previously. It uses a double-cell geometry to effect a partial separation of the sample from the convolutions of the bellows that form the outer wall of the cell. Consistent with earlier work, no evidence is found for the production of quantized vortices via the Kibble-Zurek (KZ) mechanism. Although the expansion is complete within 15ms , the second-sound velocity and attenuation continue to increase for a further approximately 60ms ; correspondingly the temperature decreases. Subsequently, the temperature rises again toward its final value as the second-sound velocity and attenuation decrease. It is shown that this unexpected behavior is apparently associated with a large-amplitude second-sound oscillation produced by the expansion, and it is suggested that the observed vortices are created by the normal fluid-superfluid counterflow that constitutes the second-sound wave. If production of large-amplitude second sound is inherent to the mechanical expansion of liquid 4He through the superfluid transition, as appears to be the case for final temperatures more than 3mK from the lambda transition, the phenomenon sets a lower bound on the density of KZ vortices that can be detected in this type of experiment. PMID:17279991

  15. Dissociation of relativistic {sup 7}Be nuclei through the {sup 3}He+{sup 4}He channel on a proton target

    SciTech Connect

    Alexandrov, Yu. A.; Peresadko, N. G. Gerasimov, S. G.; Dronov, V. A.; Pisetskaya, A. V.; Fetisov, V. N.; Kharlamov, S. P.; Shesterkina, L. N.

    2015-05-15

    The differential cross section for the interaction of {sup 7}Be nuclei with protons was measured in the momentum-transfer region extending up to a value of 0.5 GeV/c at which {sup 7}Be decay to {sup 3}He and {sup 4}He fragments was not accompanied by the emergence of other charged particles. In the momentum-transfer region extending up to about 100 MeV/c, the cross section is strongly suppressed in just the same way as in the case of the dissociation of {sup 7}Li nuclei on a proton target through the {sup 3}H+{sup 4}He channel. The total reaction cross section is 10 ± 4 mb. The mean transverse-momentum transfer in observed events is 233 ± 6 MeV/c, the dispersion of its distribution being about 63 MeV/c. The interactions in question were detected in photoemulsion irradiated with {sup 7}Be nuclei originating from a charge-exchange process involving {sup 7}Li nuclei accelerated to the momentum of 1.7 GeV/c per nucleon at the nuclotron of the Joint Institute for Nuclear Research (Dubna)

  16. Is there a stable commensurate solid phase in the second 4He layer on graphite? - path integral Monte Carlo study

    NASA Astrophysics Data System (ADS)

    Ahn, Jeonghwan; Lee, Hoonkyung; Kwon, Yongkyung

    2015-03-01

    Existence of a stable commensurate structure in the second 4He layer on graphite has been a subject of intensive experimental and theoretical studies because of its implication in the possible realization of two-dimensional supersolidity. Earlier path-integral Monte Carlo (PIMC) calculations of Pierce and Manousakis predicted a stable C4/7 commensurate structure above the first-layer 4He atoms fixed at triangular lattice sites, but Corboz et al. later showed that no commensurate phase was stable when quantum dynamics of the first-layer 4He atoms was incorporated in the PIMC calculations. On the other hand, recent heat capacity measurements of Nakamura et al. provided a strong evidence for a commensurate solid in the second 4He layer over an extended density range. Motivated by this, we have performed new PIMC calculations for the second helium layer on graphite. Unlike previous PIMC calculations where a laterally-averaged one-dimensional substrate potential was used, we here employ an anisotropic 4He-graphite potential described by a sum of the 4He-C pair potentials. With this fully-corrugated substrate potential we make more accurate description of quantum dynamics of the first-layer 4He atoms and analyze its effects on the phase diagram of the second layer.

  17. Radial sensitivity of the optical model potentials for 4He+120Sn and 6He+120Sn

    NASA Astrophysics Data System (ADS)

    Sert, Y.; Boztosun, I.

    2016-09-01

    In this paper, the radial sensitivity of the elastic scattering cross-section for the 4He and 6He on 120Sn have been examined at energies near the Coulomb barrier. We also investigate the variation of the potential radius depending on the incident energy for the 4He +120Sn and 6He +120Sn systems. Especially, we have taken care of to stay within one family for 4He +120Sn elastic scattering, i.e., using V0 real depth have not been changed by more than 20-30%.

  18. Communication: Unraveling the {sup 4}He droplet-mediated soft-landing from ab initio-assisted and time-resolved density functional simulations: Au@{sup 4}He{sub 300}/TiO{sub 2}(110)

    SciTech Connect

    Lara-Castells, María Pilar de Aguirre, Néstor F.; Stoll, Hermann; Mitrushchenkov, Alexander O.; Mateo, David; Pi, Martí

    2015-04-07

    An ab-initio-based methodological scheme for He-surface interactions and zero-temperature time-dependent density functional theory for superfluid {sup 4}He droplets motion are combined to follow the short-time collision dynamics of the Au@{sup 4}He{sub 300} system with the TiO{sub 2}(110) surface. This composite approach demonstrates the {sup 4}He droplet-assisted sticking of the metal species to the surface at low landing energy (below 0.15 eV/atom), thus providing the first theoretical evidence of the experimentally observed {sup 4}He droplet-mediated soft-landing deposition of metal nanoparticles on solid surfaces [Mozhayskiy et al., J. Chem. Phys. 127, 094701 (2007) and Loginov et al., J. Phys. Chem. A 115, 7199 (2011)].

  19. Heat capacity of {sup 4}He in Vycor near the critical coverage

    SciTech Connect

    Van Keuls, F.W.; Crowell, P.A.; Reppy, J.D.

    1993-04-01

    The authors report heat capacity measurements of {sup 4}He films in Vycor near the critical coverage. The goal of these studies is to determine whether the low temperature phase at coverages below the onset of superfluidity is a glass or an insulator with a gap. The data cover a temperature range of 5 mK to 600 mK. At the lowest temperatures, a CMN DC-SQUID thermometer is used. This thermometer contains 3 mg of CMN to minimize its heat capacity. The sensitivity at 10 mK is better than 500 pK/{radical}Hz. The CMN powder is mixed with a Ag sinter to improve thermal conductivity. The resistance thermometers mounted on the cell are found to be reliable down to 14 mK.

  20. Rapid glacial erosion at 1.8 Ma revealed by 4He/3He thermochronometry.

    PubMed

    Shuster, David L; Ehlers, Todd A; Rusmoren, Margaret E; Farley, Kenneth A

    2005-12-01

    Alpine glaciation and river incision control the topography of mountain ranges, but their relative contributions have been debated for years. Apatite 4He/3He thermochronometry tightly constrains the timing and rate of glacial erosion within one of the largest valleys in the southern Coast Mountains of British Columbia, Canada. Five proximate samples require accelerated denudation of the Klinaklini Valley initiating 1.8 +/- 0.2 million years ago (Ma). At least 2 kilometers of overlying rock were removed from the valley at >/=5 millimeters per year, indicating that glacial valley deepening proceeded >/=6 times as fast as erosion rates before approximately 1.8 Ma. This intense erosion may be related to a global transition to enhanced climate instability approximately 1.9 Ma.

  1. Studies of the 4He Nucleus in the (e,e'p) Reaction

    SciTech Connect

    Bodo Reitz

    2003-10-01

    Jefferson Lab experiment E97-111 measured the unseparated cross section for the (e,e'p) reaction on {sup 4}He at recoil momenta up to 530 {approx} MeV/c. In the plane-wave impulse approximation, many calculations predict a sharp minimum in the cross section for recoil momenta around 450 {approx} MeV/c and show that its location is sensitive to the short-range part of the internucleon potential. However, reaction dynamic effects such as final-state interactions and meson-exchange currents can obscure such a minimum. To distinguish and study these effects data were taken at several different kinematics. The preliminary results of the experiment are presented and compared to recent model calculations.

  2. Dynamic structure factor of liquid 4He across the normal-superfluid transition

    NASA Astrophysics Data System (ADS)

    Ferré, G.; Boronat, J.

    2016-03-01

    We have carried out a microscopic study of the dynamic structure factor of liquid 4He across the normal-superfluid transition temperature using the path integral Monte Carlo method. The ill-posed problem of the inverse Laplace transform, from the imaginary-time intermediate scattering function to the dynamic response, is tackled by stochastic optimization. Our results show a quasiparticle peak and a small and broad multiphonon contribution. In spite of the lack of strength in the collective peaks, we clearly identify the rapid dropping of the roton peak amplitude when crossing the transition temperature Tλ. Other properties such as the static structure factor, static response, and one-phonon contribution to the response are also calculated at different temperatures. The changes of the phonon-roton spectrum with the temperature are also studied. An overall agreement with available experimental data is achieved.

  3. Disappearance of Roton Propagation in Superfluid {sup 4}He at T{sub {lambda}}

    SciTech Connect

    Svensson, E.C.; Montfrooij, W.; de Schepper, I.M.

    1996-11-01

    Using neutron scattering, we determine the dynamic structure factor {ital S}({ital q},{nu}) of liquid {sup 4}He for the roton wave number {ital q}=2.0{sup {minus}1} as a function of frequency {nu} at constant density 0.1715 gcm{sup {minus}3} and for ten temperatures in the range 1.08{le}{ital T}{le}2.00 K, primarily near the superfluid transition temperature {ital T}{sub {lambda}}=1.9202 K. The {lambda} transition is marked by a complete softening of the roton mode and a rapid decrease in lifetime. This change is continuous with temperature, and we find no evidence for a new mode appearing as one enters the superfluid phase, as has been proposed on the basis of theoretical considerations. {copyright} {ital 1996 The American Physical Society.}

  4. Critical Scaling Properties at the Superfluid Transition of {sup 4}He in Aerogel

    SciTech Connect

    Nikolaou, Marios; Wallin, Mats; Weber, Hans

    2006-12-01

    We study the superfluid transition of {sup 4}He in aerogel by Monte Carlo simulations and finite size scaling analysis. Aerogel is a highly porous silica glass, which we model by a diffusion limited cluster aggregation model. The superfluid is modeled by a three dimensional XY model, with excluded bonds to sites on the aerogel cluster. We obtain the correlation length exponent {nu}=0.73{+-}0.02, in reasonable agreement with experiments and with previous simulations. For the heat capacity exponent {alpha}, both experiments and previous simulations suggest deviations from the Josephson hyperscaling relation {alpha}=2-d{nu}. In contrast, our Monte Carlo results support hyperscaling with {alpha}=-0.2{+-}0.05. We suggest a reinterpretation of the experiments, which avoids scaling violations and is consistent with our simulation results.

  5. {sup 3}He+{sup 4}He {yields} {sup 7}Be astrophysical S factor

    SciTech Connect

    Brown, T. A. D.; Bordeanu, C.; Snover, K. A.; Storm, D. W.; Melconian, D.; Sallaska, A. L.; Sjue, S. K. L.; Triambak, S.

    2007-11-15

    We present precision measurements of the {sup 3}He+{sup 4}He {yields} {sup 7}Be reaction in the range E{sub c.m.}=0.33 to 1.23 MeV using a small gas cell and detection of both prompt {gamma} rays and {sup 7}Be activity. Our prompt and activity measurements are in good agreement within the experimental uncertainty of several percent. We find S(0)=0.595{+-}0.018 keV b from fits of the Kajino theory to our data. We compare our results with published measurements, and we discuss the consequences for Big Bang Nucleosynthesis and for solar neutrino flux calculations.

  6. Experimental study of nanofluidics and phase transitions of normal and superfluid 4He

    NASA Astrophysics Data System (ADS)

    Velasco, Angel Enriques

    This thesis addresses the experimental results of two different research topics. The first is the experimental work of pressure driven flows in the smallest, single nanotubes ever investigated. The nanotube boundary conditions and slip lengths from argon, nitrogen, water, and helium experiments were analyzed and compared to macroscopic boundary conditions. The second research topic discusses the work on ellipsometric and quartz microbalance measurements of the 2D superfluid phase diagram of 4He on alkali substrates. Ellipsometric results of sodium on HOPG provide the first evidence of the existence of the 2D critical point on an intermediate strength substrate. Pressure driven flows through single nanopores and microtubes were measured with a calibrated mass spectrometer with pressure drops up to 30 Atm. The nanopores were between 30 nm to 600 nm in diameter and etched in mica and PET membranes of several microns thickness. Microtubes several inches long of fused quartz and nickel material were tested with diameters between 1.8 micron and 25 micron. For 4He and argon gas we observed the flow transition between the free molecular and continuum regimes at 293 K and 77 K. No discrepancy between the macroscopic theory and the 30 nm nanopore data was found. Because of the exceptionally low viscosity of gaseous helium the laminar-turbulent transition could also be observed within these submicron channels. The small viscosity of 4He was too small to dampen inertial effects at a Reynolds number of 2000. In addition to single phase gas flows, our experimental technique also allows us to investigate flows in which the nano or micro scale pipe is either partially or completely filled with liquids. The position of the intrinsic liquid/vapor interface was important for understanding this type of flow. Strong evaporation and cooling at the liquid-vapor interface can lead to freezing for conventional fluids such as nitrogen and water, which in turn leads to complex intermittent

  7. A predictive theory for elastic scattering and recoil of protons from 4He

    DOE PAGES

    Hupin, Guillaume; Quaglioni, Sofia; Navratil, Petr

    2014-12-08

    Low-energy cross sections for elastic scattering and recoil of protons from 4He nuclei (also known as α particles) are calculated directly by solving the Schrodinger equation for five nucleons interacting through accurate two- and three-nucleon forces derived within the framework of chiral effective field theory. Precise knowledge of these processes at various proton backscattering/recoil angles and energies is needed for the ion-beam analysis of numerous materials, from the surface layers of solids, to thin films, to fusion-reactor materials. Indeed, the same elastic scattering process, in two different kinematic configurations, can be used to probe the concentrations and depth profiles ofmore » either hydrogen or helium. Furthermore, we compare our results to available experimental data and show that direct calculations with modern nuclear potentials can help to resolve remaining inconsistencies among data sets and can be used to predict these cross sections when measurements are not available.« less

  8. Ac vortex-dependent torsional oscillation response and onset temperature T0 in solid 4He.

    PubMed

    Penzev, Andrey; Yasuta, Yoshinori; Kubota, Minoru

    2008-08-01

    Detailed studies of ac velocity V_{ac} and T dependence of torsional oscillator responses of solid 4He are reported. A characteristic onset temperature T_{0} approximately 0.5 K is found, below which a significant V_{ac}-dependent change occurs in the energy dissipation for the samples at approximately 32 bar and for one at 49 bar. A V_{ac} dependence of the so-called "nonclassical rotational inertia" fraction also appears below approximately T_{0}. The log(V_{ac}) linear dependence, which suggests involvement of quantized vorticies, was examined in the nonclassical rotational inertia fraction. We find a common 1/T;{2} dependence for this linear slope change in all of the samples for 30

  9. Relaxation dynamics of spindodal decomposition in superfluid ^3He-^4He mixtures

    NASA Astrophysics Data System (ADS)

    Chay, Terrence Y.; Goldenfeld, Nigel; Bauer, Gregory H.; Ceperley, David M.

    1998-03-01

    We study the dynamics of the Hohenberg-Nelson system(P.C. Hohenberg and David R. Halperin, Phys. Rev. B 20):2665 (1979). for ^3He-^4He mixtures after a quench using a mesoscopic cell dynamical systems (CDS) model. The spinodal region is characterized by maximal growth at a single nonzero wave vector which scales with time. Because CDS exploits universality to avoid taking Δ x and Δ t to infinitesimals, rapid simulations are possible on large systems making it an ideal way to find such scaling behavior. Using thermodynamic properties obtained from experiement and exactly calculated from path integral monte carlo studies, one can obtain the workable CDS phenomenological parameters to do time evolution studies of large-scale mixtures.

  10. Nuclear Transparency with the gamma + n -> pi- + p Process in 4He

    SciTech Connect

    Dipangkar Dutta; Feng Xiong; Lingyan Zhu; John Arrington; Todd Averett; Elizabeth Beise; John Calarco; Ting Chang; Jian-Ping Chen; Eugene Chudakov; Marius Coman; Benjamin Clasie; Christopher Crawford; Sonja Dieterich; Frank Dohrmann; Kevin Fissum; Salvatore Frullani; Haiyan Gao; Ronald Gilman; Charles Glashausser; Javier Gomez; Kawtar Hafidi; Jens-Ole Hansen; Douglas Higinbotham; R.J. Holt; Cornelis De Jager; Xiaochao Zheng; X. Jiang; Edward Kinney; Kevin Kramer; Gerfried Kumbartzki; John LeRose; Nilanga Liyanage; David Mack; Pete Markowitz; Kathy McCormick; Zein-Eddine Meziani; Robert Michaels; J. Mitchell; Sirish Nanda; David Potterveld; Ronald Ransome; Paul Reimer; Bodo Reitz; Arunava Saha; Elaine Schulte; Charles Seely; Simon Sirca; Steffen Strauch; Vincent Sulkosky; Branislav Vlahovic; Lawrence Weinstein; Krishni Wijesooriya; Claude Williamson; Bogdan Wojtsekhowski; Hong XIANG; Wang Xu; J. Zeng

    2003-08-01

    We have measured the nuclear transparency of the fundamental process {gamma} n {yields} {pi}{sup -} p in {sup 4}He. These measurements were performed at Jefferson Lab in the photon energy range of 1.6 to 4.5 GeV and at {theta}{sub cm}{sup {pi}} = 70{sup o} and 90{sup o}. These measurements are the first of their kind in the study of nuclear transparency in photoreactions. They also provide a benchmark test of Glauber calculations based on traditional models of nuclear physics. The transparency results suggest deviations from the traditional nuclear physics picture. The momentum transfer dependence of the measured nuclear transparency is consistent with Glauber calculations which include the quantum chromodynamics phenomenon of color transparency.

  11. Dynamics of {sup 3}He impurities in {sup 4}He films

    SciTech Connect

    Clements, B.E. |; Krotscheck, E. |; Saarela, M.

    1995-08-01

    Using a microscopic variational theory the authors calculate the binding energy of {sup 3}He impurities in films of {sup 4}He absorbed to a graphite substrate. Without adjustable parameters, they obtain excellent agreement with the experimental binding energies for the ground state of the {sup 3}He impurity. To calculate excited states, they then introduce a time-dependent variational wave function. In that way, the impurity acquires a hydrodynamic effective mass for its motion parallel to the surface due to hydrodynamic backflow. Excited states have a finite lifetime. When these effects are included, both the energy of the first excited state of the impurity, and the effective mass of the ground state, also agree well with experimental data.

  12. Response functions of imaging plates to photons, electrons and {sup 4}He particles

    SciTech Connect

    Bonnet, T.; Denis-Petit, D.; Gobet, F.; Hannachi, F.; Tarisien, M.; Versteegen, M.; Aléonard, M. M.

    2013-10-15

    Imaging plates from Fuji (BAS-SR, MS, and TR types) are phosphor films routinely used in ultra high intensity laser experiments. However, few data are available on the absolute IP response functions to ionizing particles. We have previously measured and modeled the IP response functions to protons. We focus here on the determination of the responses to photons, electrons, and {sup 4}He particles. The response functions are obtained on an energy range going from a few tens of keV to a few tens of MeV and are compared to available data. The IP sensitivities to the different ionizing particles demonstrate a quenching effect depending on the particle stopping power.

  13. Microscopic optical model calculations of 4He, 12C-nucleus absorption cross sections

    NASA Technical Reports Server (NTRS)

    Dubey, R. R.; Khandelwal, G. S.; Cucinotta, F. A.; Wilson, J. W.

    1996-01-01

    Calculations of absorption cross sections using a microscopic first-order optical potential for heavy-ion scattering are compared with experiments. In-medium nucleon-nucleon (NN) cross sections were used to calculate the two-body scattering amplitude. A medium-modified first-order optical potential was obtained for heavy-ion scattering using the in-medium two-body scattering amplitude. A partial wave expansion of the Lippmann-Schwinger equation in momentum space was used to calculate the absorption cross sections for various systems. The results are presented for the absorption cross sections for 4He-nucleus and 12C-nucleus scattering systems and are compared with the experimental values in the energy range 18-83A MeV. The use of the in-medium NN cross sections is found to result in significant reduction of the free space absorption cross sections in agreement with experiment.

  14. Russell Donnelly's last legacy: Pursuing grid turbulence in superfluid 4He

    NASA Astrophysics Data System (ADS)

    Ihas, Gary; Yang, Jihee

    2015-11-01

    Quantum turbulence, a tangle of quantized vortex lines in a superfluid, may hold significant keys to understanding all types of turbulence. Russell Donnelly pioneered this line of research, beginning with studies of grid turbulence probed by second sound. The apparatus built by Russell and his students, with significant up-grades, is now being used at the University of Florida to continue his work on decaying grid turbulence in superfluid 4He. The Oregon work used a 1cm wide square channel, while the Florida work has been in both 1 cm and 5 cm square channels. The larger channel allows detailed study of the increase in eddy size before saturation at the channel walls during the decay process. Power law fits of the turbulence decay in time allow comparison with theory, work intended to be Russell Donnelly's last experiment. Supported in part by US NSF #1007937.

  15. Theoretical analysis of the anomalous spectral splitting of tetracene in 4He droplets.

    PubMed

    Whitley, Heather D; DuBois, Jonathan L; Whaley, K Birgitta

    2011-06-30

    We present a theoretical analysis of the electronic absorption spectra of tetracene in (4)He droplets based on many-body quantum simulations. Using the path integral ground state approach, we calculate one- and two-body reduced density matrices of the most strongly localized He atoms near the molecule surface and use these to investigate the helium ground-state quantum coherence and correlations when tetracene is in its electronic ground and excited states. We identify a trio of quasi-one-dimensional, strongly localized atoms adsorbed along the long axis of the molecule that show some quantum coherence among themselves but far less with the remaining solvating helium. We evaluate the single-particle natural orbitals of the localized He atoms by diagonalization of the one-body density matrix and use these to construct single- and many-particle solvating helium basis states with which the zero-phonon spectral features of the tetracene-(4)He(N) absorption spectrum are then calculated. The absorption spectrum resulting from the three-body density matrix for the strongly bound trio of helium atoms is in very good agreement with the experimental data, accounting quantitatively for the anomalous splitting of the zero-phonon line [Hartmann, M.; Lindinger, A.; Toennies, J. P.; Vilesov, A. F. Chem. Phys. 1998, 239, 139; Krasnokutski, S.; Rouillé, G.; Huisken, F. Chem. Phys. Lett. 2005, 406, 386]. Our results indicate that the combination of strong localization and the quasi-one-dimensional nature of trios of helium atoms adsorbed along the long axis of tetracene leads to a quantum coherent, yet highly correlated ground state for the helium density closest to the molecule. The spectroscopic analysis shows that this feature accounts quantitatively for the anomalous splittings and hitherto unexplained fine structure observed in the absorption spectra of tetracene and suggests that it may be responsible for the corresponding zero-phonon splittings in other quasi

  16. Distinguishing 3He and 4He with the Electron Proton Telescope (EPT) on Solar Orbiter

    NASA Astrophysics Data System (ADS)

    Boden, S.; Kulkarni, S. R.; Steinhagen, J.; Tammen, J.; Martin-Garcia, C.; Wimmer-Schweingruber, R. F.; Boettcher, S. I.; Seimetz, L.; Ravanbakhsh, A.; Elftmann, R.; Schuster, B.; Kulemzin, A.; Kolbe, S.; Mahesh, Y.; Knieriem, V.; Yu, J.; Kohler, J.; Panitzsch, L.; Terasa, C.; Boehm, E.; Rodriguez-Pacheco, J.; Prieto, M.; Gomez-Herrero, R.

    2015-12-01

    The Electron Proton Telescope (EPT) is one of the sensors of the Energetic Particle Detector (EPD) for the Solar Orbiter mission, which will provide key measurements to address particle acceleration at and near the Sun. The EPD suite consists of four different sensors (STEP, SIS, EPT and HET) which together will resolve the energetic particle spectrum from 2 keV to 20 MeV for electrons, 3 keV to 100 MeV for protons and circa 100 keV/nuc to 100 MeV/nuc for heavier ions.EPT itself is primarily designed to cleanly separate and measure electrons in the energy range from 20 - 400 keV and protons from 20 - 7000 keV. To achieve this, EPT uses two back-to-back solid state detectors with a magnet system to deflect electrons on one side and a Polyimide foil to stop protons below ~400 keV on the other side. The two detectors then serve as each other's anti-coincidence. Additionally this setup also allows us to measure penetrating particles with deposited energies in the 1 MeV to 40 MeV range. Looking at the ratio of deposited energy in the two detectors versus total deposited energy allows us to differentiate between protons and alpha particles. Distinguishing 3He from 4He will be challenging, but possible provided good knowledge of the instrument, high-fidelity modeling and a precise calibration of EPT. Here, we will present feasibility studies leading to a determination of the 3He / 4He ratio with EPT.

  17. Phonon-roton modes of liquid 4He beyond the roton in MCM-41

    SciTech Connect

    Azuah, Richard T; Omar Diallo, Souleymane; Adams, Mark A.; Kirichek, Oleg; Glyde, Henry R

    2013-01-01

    We present neutron scattering measurements of the phonon-roton (P-R) mode of superfluid 4He confined in 47 A MCM-41 at T = 0.5 K at wave vectors, Q, beyond the roton wave vector (QR = 1.92 A-1). Measurements beyond the roton require access to high wave vectors (up to Q = 4 A-1) with excellent energy resolution and high statistical precision. The present results show for the first time that at T = 0.5 K the P-R mode in MCM-41 extends out to wave-vector Q 3.6 A-1 with the same energy and zero width (within precision) as observed in bulk superfluid 4He. Layer modes in the roton region are also observed. Specifically, the P-R mode energy, !Q, increases with Q for Q > QR and reaches a plateau at a maximum energy !Q = 2 where is the roton energy, = 0.74 0.01 meV in MCM-41. This upper limit means the P-R mode decays to two rotons when its energy exceeds 2 . It also means that the P-R mode does not decay to two layers modes. If the P-R could decay to two layer modes, !Q would plateau at a lower energy, !Q = 2 L where L = 0.60 meV is the energy of the roton like minimum of the layer mode. The observation of the P-R mode with energy up to 2 shows that the P-R mode and the layer modes are independent modes with apparently little interaction between them.

  18. Probing Liquid ^4He with Quartz Tuning Forks Using a Novel Multifrequency Lock-in Technique

    NASA Astrophysics Data System (ADS)

    Bradley, D. I.; Haley, R. P.; Kafanov, S.; Noble, M. T.; Pickett, G. R.; Tsepelin, V.; Vonka, J.; Wilcox, T.

    2016-09-01

    We report on a novel technique to measure quartz tuning forks, and possibly other vibrating objects, in a quantum fluid using a multifrequency lock-in amplifier. The multifrequency technique allows to measure the resonance curve of a vibrating object much faster than a conventional single frequency lock-in amplifier technique. Forks with resonance frequencies of 12 kHz and 16 kHz were excited and measured electro-mechanically either at a single frequency or at up to 40 different frequencies simultaneously around the same mechanical mode. The response of each fork was identical for both methods and validates the use of the multifrequency lock-in technique to probe properties of liquid helium at low fork velocities. Using both methods we measured the resonance frequency and drag of two 25-μ m-wide quartz tuning forks immersed in liquid ^4He in the temperature range from 4.2 K to 1.5 K at saturated vapour pressure. The damping and shift of resonance frequency experienced by both tuning forks at low velocities are well described by hydrodynamic contributions in the framework of the two-fluid model. The sensitivity of the 25-μ m-wide tuning forks is larger compared to similar 75-μ m-wide forks and in combination with the faster multifrequency lock-in technique could be used to improve thermometry in liquid ^4He. The multifrequency technique could also be used for studies of the onset of non-linear phenomena such as quantum turbulence and cavitation in superfluids.

  19. {sup 4}He liquid-vapor interface below 1 K studied using x-ray reflectivity

    SciTech Connect

    Penanen, Konstantin; Fukuto, Masafumi; Heilmann, Ralf K.; Silvera, Isaac F.; Pershan, Peter S.

    2000-10-01

    The free surface of thin films of liquid helium adsorbed on a solid substrate has been studied using x-ray reflectivity. The film thickness and interfacial profile are extracted from the angular dependence of measured interference between signals reflected from the liquid-vapor and liquid-substrate interfaces. Polished silicon wafers, chemically cleaned and passivated, were used as substrates. Results are reported for measurements for {sup 4}He films 35 to 130 Aa thick in the temperature range 0.44 to 1.3 K. The 10%/90% interfacial width for temperature T=0.45 K varies from 5.3{+-}0.5 Aa for 36{+-}1.5 Aa thick films to 6.5{+-}0.5 Aa for 125{+-}1.5 Aa thick films. The profile width at zero temperature should not differ significantly from that measured at T=0.45 K. For T=1.22 K, the width is 7.8{+-}1.0 Aa.

  20. Determination of the effective kinematic viscosity for the decay of quasiclassical turbulence in superfluid 4He

    NASA Astrophysics Data System (ADS)

    Gao, J.; Guo, W.; Vinen, W. F.

    2016-09-01

    The energy dissipation of quasiclassical homogeneous turbulence in superfluid 4He (He II) is controlled by an effective kinematic viscosity ν', which relates the energy decay rate d E /d t to the density of quantized vortex lines L as d E /d t =-ν'(κL ) 2 . The precise value of ν' is of fundamental importance in developing our understanding of the dissipation mechanism in He II, and it is also needed in many high-Reynolds-number turbulence experiments and model testing that use He II as the working fluid. However, a reliable determination of ν' requires the measurements of both E (t ) and L (t ) , which was never achieved. Here we discuss our study of the quasiclassical turbulence that emerges in the decay of thermal counterflow in He II above 1 K. We were able to measure E (t ) by using a recently developed flow-visualization technique and L (t ) via second-sound attenuation. We report the ν' values in a wide temperature range determined from a comparison of the time evolution of E (t ) and L (t ) .

  1. Time-resolved study of laser initiated shock wave propagation in superfluid 4He

    NASA Astrophysics Data System (ADS)

    Garcia, Allan; Buelna, Xavier; Popov, Evgeny; Eloranta, Jussi

    2016-09-01

    Intense shock waves in superfluid 4He between 1.7 and 2.1 K are generated by rapidly expanding confined plasma from laser ablation of a metal target immersed in the liquid. The resulting shock fronts in the liquid with initial velocities up to ca. Mach 10 are visualized by time-resolved shadowgraph photography. These high intensity shocks decay within 500 ns into less energetic shock waves traveling at Mach 2, which have their lifetime in the microsecond time scale. Based on the analysis using the classical Rankine-Hugoniot theory, the shock fronts created remain in the solid phase up to 1 μs and the associated thermodynamic state appears outside the previously studied region. The extrapolated initial shock pressure of 0.5 GPa is comparable to typical plasma pressures produced during liquid phase laser ablation. A secondary shock originating from fast heat propagation on the metal surface is also observed and a lower limit estimate for the heat propagation velocity is measured as 7 × 104 m/s. In the long-time limit, the high intensity shocks turn into liquid state waves that propagate near the speed of sound.

  2. Third Sound Generation in Superfluid 4He Films Adsorbed on Multiwall Carbon Nanotubes

    NASA Astrophysics Data System (ADS)

    Iaia, Vito; Menachekanian, Emin; Williams, Gary

    2014-03-01

    A technique is developed for generating third sound in superfluid 4He films coating the surface of multiwall carbon nanotubes. Third sound is a thickness and temperature wave of the helium film, and in our case we detect the temperature oscillations with a carbon resistance bolometer. The nanotubes are packed in an annular resonator that is vibrated with a mechanical shaker assembly consisting of a permanent magnet mounted on springs, and surrounded by a superconducting coil. The coil is driven with an oscillating current, vibrating the cell at that frequency. Sweeping the drive frequency over the range 100-200 Hz excites the resonant third sound mode of the cell, seen as a high-Q signal in the FFT analysis of the bolometer signal. A problem with our original cell was that the mechanical drive would also shake the dilution refrigerator cooling the cell to low temperatures, and increasing the drive would start to heat up the refrigerator and the cell, which were rigidly coupled together. A new configuration now suspends the cell as a pendulum on a string, with thermal contact made by copper wires. Piezo sensor measurements show this reduces the vibration reaching the refrigerator by two orders of magnitude, which should allow measurements at lower temperatures.

  3. Operator evolution for ab initio electric dipole transitions of 4He

    DOE PAGES

    Schuster, Micah D.; Quaglioni, Sofia; Johnson, Calvin W.; Jurgenson, Eric D.; Navartil, Petr

    2015-07-24

    A goal of nuclear theory is to make quantitative predictions of low-energy nuclear observables starting from accurate microscopic internucleon forces. A major element of such an effort is applying unitary transformations to soften the nuclear Hamiltonian and hence accelerate the convergence of ab initio calculations as a function of the model space size. The consistent simultaneous transformation of external operators, however, has been overlooked in applications of the theory, particularly for nonscalar transitions. We study the evolution of the electric dipole operator in the framework of the similarity renormalization group method and apply the renormalized matrix elements to the calculationmore » of the 4He total photoabsorption cross section and electric dipole polarizability. All observables are calculated within the ab initio no-core shell model. Furthermore, we find that, although seemingly small, the effects of evolved operators on the photoabsorption cross section are comparable in magnitude to the correction produced by including the chiral three-nucleon force and cannot be neglected.« less

  4. Theory of neutron scattering from thermally excited quasiparticles in superfluid 4He

    NASA Astrophysics Data System (ADS)

    Griffin, A.; Talbot, E.

    1981-11-01

    We present the first detailed theoretical study of the inelastic neutron scattering contribution Sth(Q-->,ω) from thermally excited quasiparticles in superfluid 4He, with emphasis on the low-Q collisionless limit. In the temperature region where rotons are the dominant excitation, our results for Sth(Q-->,ω) scale with Landau's normal fluid density. We argue that Sth(Q-->,ω) is the origin of the broad temperature-dependent continuum which Woods and Svensson (1978) have observed at temperatures above about 1.7 K. Our specific model calculations of Sth(Q-->,ω) are based on evaluating the regular part of the longitudinal momentum current-current correlation function within the Bogoliubov approximation, but the experimental quasiparticle (roton) spectrum is used in our numerical calculations. Our expression satisfies the normal fluid f-sum rule in the long-wavelength collisionless limit and is in essential agreement with the general picture suggested by Pines and Nozières in 1964. Our present theory involves several approximations which probably limit its validity to Q<~0.5 Å-1. Some generalizations to deal with the larger values of Q studied by Woods and Svensson are briefly discussed.

  5. Path integral studies of the rotations of methane and its heavier isotopomers in 4He nanoclusters.

    PubMed

    Markovskiy, N D; Mak, C H

    2009-08-13

    Path integral Monte Carlo simulations have been carried out to study the rotations of a methane molecule and its heavier isotopomers inside a small cluster of 4He atoms at 0.3 K in order to determine how the renormalization in the methane's rotational constant is related to the quantum statistics and superfluidity of the helium shell. By changing the mass of the hydrogens and systematically varying the moment of inertia of the methane, we were able to study the effects of its rotations on the quantum statistics of the helium atoms and their countereffects on the methane's effective rotational constant. The renormalized rotational constant depends strongly on the intrinsic moment of inertia of the methane. A heavy probe favors strong templating of the helium density as well as a large renormalization in the probe's rotational constant, but a light probe shows almost no effect on the shell density or the effective rotational constant. These results suggest that in order to fully understand the superfluidity of the helium shell, the probe must be treated as an integral part of the system. We rationalize the findings in terms of a rotational smearing effect and suggest that there is no clearly quantifiable relationship between the superfluid fraction of the shell and the renormalized rotational constant of the probe for cases where the probe molecule is either light or has weak anisotropic interactions with the helium atoms. PMID:19618956

  6. Polarized liquid3He in a4He circulating dilution refrigerator

    NASA Astrophysics Data System (ADS)

    Rodrigues, Alexandre; Vermeulen, Gerard

    1995-10-01

    We have used a4He circulating dilution refrigerator to produce cold liquid3He with a steady state out-of-equilibrium nuclear spin polarization. Polarizations on the order of 15% (more than 7 times higher than the equilibrium polarization in the external field of 6.6 T) have been obtained in the mixing chamber of the refrigerator at temperatures between 10 and 15 mK. The polarization is enhanced at high pressure because the molar susceptibility of concentrated3He is larger than that of the dilute phase. The polarization exchange between the dilute and concentrated phases (in direct contact in the heat exchanger of the refrigerator) amplifies the enhancement. The polarization diminishes below a pressure of 2.6 bar. This allows us to scale and reinterpret susceptibility data of the dilute phase1 in combination with the effective mass deduced from osmotic pressure measurements2. We find 1+F{0/a} = 0.89±1% on the phase separation line in the pressure range 0 20 bar.

  7. Fluid pinch-off in superfluid and normal {sup 4}He

    SciTech Connect

    Burton, J. C.; Rutledge, J. E.; Taborek, P.

    2007-03-15

    We present frames from high-speed videos of the pinch-off of liquid {sup 4}He droplets. The temperature of the fluid droplets ranged from 1.33 K to 4.8 K, and the size of the drops was proportional to the temperature-dependent capillary length. We observed no qualitative difference between pinch-off in the normal and superfluid states. In both cases, the shape of the fluid in the final stages of pinch-off resembles a cone piercing a sphere, which is typical of other low-viscosity fluids. The evolution of the minimum neck radius r{sub min} can be characterized by power laws r{sub min}{proportional_to}{tau}{sup n}, where {tau} is the time remaining until pinch-off occurs. In the regime near pinch-off, the data from image analysis are consistent with n=2/3. The data at the beginning of the pinch process when the neck is of the order of the capillary length are also described by n=2/3, but with a different proportionality factor. There is an intermediate crossover regime characterized by n=2/5.

  8. Copper dimer interactions on a thermomechanical superfluid {sup 4}He fountain

    SciTech Connect

    Popov, Evgeny; Eloranta, Jussi

    2015-05-28

    Laser induced fluorescence imaging and frequency domain excitation spectroscopy of the copper dimer (B{sup 1}Σ{sub g}{sup +}←X{sup 1}Σ{sub u}{sup +}) in thermomechanical helium fountain at 1.7 K are demonstrated. The dimers penetrate into the fountain provided that their average propagation velocity is ca. 15 m/s. This energy threshold is interpreted in terms of an imperfect fountain liquid-gas interface, which acts as a trap for low velocity dimers. Orsay-Trento density functional theory calculations for superfluid {sup 4}He are used to characterize the dynamics of the dimer solvation process into the fountain. The dimers first accelerate towards the fountain surface and once the surface layer is crossed, they penetrate into the liquid and further slow down to Landau critical velocity by creating a vortex ring. Theoretical lineshape calculations support the assignment of the experimentally observed bands to Cu{sub 2} solvated in the bulk liquid. The vibronic progressions are decomposed of a zero-phonon line and two types of phonon bands, which correlate with solvent cavity interface compression (t < 200 fs) and expansion (200 < t < 500 fs) driven by the electronic excitation. The presented experimental method allows to perform molecular spectroscopy in bulk superfluid helium where the temperature and pressure can be varied.

  9. Evidence for intertwined superfluid and density wave order in two dimensional 4He

    NASA Astrophysics Data System (ADS)

    Saunders, John

    2015-03-01

    We report the identification of a new state of quantum matter with intertwined superfluid and density wave order in a system of two dimensional bosons subject to a triangular lattice potential. Using a torsional oscillator we have measured the response of the second atomic layer of 4He adsorbed on the surface of graphite over a wide temperature range down to 2 mK. Superfluidity is observed over a narrow range of film densities, emerging suddenly and collapsing towards a quantum critical point, near to layer completion where a Mott insulating phase is predicted to form. The unusual temperature dependence of the superfluid density in the T --> 0 limit and the absence of a clear superfluid onset temperature are explained, self-consistently, by an ansatz for the excitation spectrum, reflecting density wave order, and a quasi-condensate wavefunction breaking both gauge and translational symmetry. In collaboration with Jan Nyeki, Anastasia Phillis, Andrew Ho, Derek Lee, Piers Coleman, Jeevak Parpia, Brian Cowan. Supported by EPSRC (U.K) EP/H048375/1.

  10. Improvement of the Spatial Amplitude Isotropy of a ^4He Magnetometer Using a Modulated Pumping Beam

    NASA Astrophysics Data System (ADS)

    Chéron, B.; Gilles, H.; Hamel, J.; Moreau, O.; Noël, E.

    1997-08-01

    Optically pumped magnetometers are scalar magnetometers. Contrary to vectoriel magnetometers, they measure the total magnetic field whatever the direction of the sensor. However, for some orientations of the magnetometer with respect to the magnetic field direction, the resonant signal vanishes and the measurement is impossible. In this paper we present a simple solution to reduce the amplitude spatial anisotropy and apply it to a ^4He magnetometer developed in our Laboratory. Les magnétomètres à pompage optique sont des magnétomètres scalaires. Contrairement aux magnétomètres vectoriels, ils mesurent le module du champ magnétique quelle que soit l'orientation du capteur dans l'espace. Cependant, pour certaines orientations du magnétomètre par rapport à la direction du champ à mesurer, l'amplitude du signal de résonance s'annule et la mesure devient impossible. Dans cet article, nous présentons une solution simple pour réduire l'anisotropie spatiale d'amplitude et nous l'appliquons à un magnétomètre à hélium-4 développé dans notre Laboratoire.

  11. One-Dimensional Liquid ^{4}He: Dynamical Properties beyond Luttinger-Liquid Theory.

    PubMed

    Bertaina, G; Motta, M; Rossi, M; Vitali, E; Galli, D E

    2016-04-01

    We compute the zero-temperature dynamical structure factor of one-dimensional liquid ^{4}He by means of state-of-the-art quantum Monte Carlo and analytic continuation techniques. By increasing the density, the dynamical structure factor reveals a transition from a highly compressible critical liquid to a quasisolid regime. In the low-energy limit, the dynamical structure factor can be described by the quantum hydrodynamic Luttinger-liquid theory, with a Luttinger parameter spanning all possible values by increasing the density. At higher energies, our approach provides quantitative results beyond the Luttinger-liquid theory. In particular, as the density increases, the interplay between dimensionality and interaction makes the dynamical structure factor manifest a pseudo-particle-hole continuum typical of fermionic systems. At the low-energy boundary of such a region and moderate densities, we find consistency, within statistical uncertainties, with predictions of a power-law structure by the recently developed nonlinear Luttinger-liquid theory. In the quasisolid regime, we observe a novel behavior at intermediate momenta, which can be described by new analytical relations that we derive for the hard-rods model. PMID:27081985

  12. 4He+n+n continuum within an ab initio framework

    DOE PAGES

    Romero-Redondo, Carolina; Quaglioni, Sofia; Navratil, Petr; Hupin, Guillaume

    2014-07-16

    In this study, the low-lying continuum spectrum of the 6He nucleus is investigated for the first time within an ab initio framework that encompasses the 4He+n+n three-cluster dynamics characterizing its lowest decay channel. This is achieved through an extension of the no-core shell model combined with the resonating-group method, in which energy-independent nonlocal interactions among three nuclear fragments can be calculated microscopically, starting from realistic nucleon-nucleon interactions and consistent ab initio many-body wave functions of the clusters. The three-cluster Schrödinger equation is solved with three-body scattering boundary conditions by means of the hyperspherical-harmonics method on a Lagrange mesh. Using amore » soft similarity-renormalization-group evolved chiral nucleon-nucleon potential, we find the known Jπ = 2+ resonance as well as a result consistent with a new low-lying second 2+ resonance recently observed at GANIL at ~2.6 MeV above the He6 ground state. We also find resonances in the 2–, 1+, and 0– channels, while no low-lying resonances are present in the 0+ and 1– channels.« less

  13. Generalized theory of double-resonance optical pumping of {sup 4}He

    SciTech Connect

    Plante, Michael K.; MacFarlane, Duncan L.; McGregor, Douglas D.; Slocum, Robert E.; Sampson, William M.; Brown, Andy W.

    2010-07-15

    We present extensions to the theory of double-resonance laser pumping of {sup 4}He in the context of magnetometer instrumentation. This extended theory allows for arbitrary optical polarization, magnetic resonance (H{sub 1}) coil orientation, and overall instrument orientation relative to the ambient magnetic field. Steady-state solutions are presented for portions of the extended parameter space. These calculations are used to analyze the shot-noise-limited sensitivities for helium magnetometers for selected parameter values, and we find that linearly polarized light can have a relatively simple orientational dependence for a particular choice of angle between the H{sub 1} coils and the light polarization vector. Calculations are also compared to experimentally measured magnetic resonance curves, and a shot-noise limit on sensitivity of 6 fT/{radical}(Hz) is determined for a particular magnetometer apparatus using a cell 2.4 cm in diameter and 7.5 cm in length. This extended theory can be utilized to select optimal operational parameter values and obtain ideal sensitivities for helium magnetometers.

  14. Electromagnetic and neutral-weak response functions of 4He and 12C

    NASA Astrophysics Data System (ADS)

    Lovato, A.; Gandolfi, S.; Carlson, J.; Pieper, Steven C.; Schiavilla, R.

    2015-06-01

    Background: A major goal of nuclear theory is to understand the strong interaction in nuclei as it manifests itself in terms of two- and many-body forces among the nuclear constituents, the protons and neutrons, and the interactions of these constituents with external electroweak probes via one- and many-body currents. Purpose: The objective of the present work is to calculate the quasielastic electroweak response functions in light nuclei within the realistic dynamical framework outlined above. These response functions determine the inclusive cross section as function of the lepton momentum and energy transfers. Methods: Their ab initio calculation is a very challenging quantum many-body problem, since it requires summation over the entire excitation spectrum of the nucleus and inclusion in the electroweak currents of one- and many-body terms. Green's functions Monte Carlo methods allow one to circumvent both difficulties by computing the response in imaginary time (the so-called Euclidean response) and hence summing implicitly over the bound and continuum states of the nucleus, and by implementing specific algorithms designed to deal with the complicated spin-isospin structure of nuclear many-body operators. Results: Theoretical predictions for 4He and 12C, confirmed by experiment in the electromagnetic case, show that two-body currents generate excess transverse strength from threshold to the quasielastic to the dip region and beyond. Conclusions: These results challenge the conventional picture of quasielastic inclusive scattering as being largely dominated by single-nucleon knockout processes.

  15. Interaction of ions, atoms, and small molecules with quantized vortex lines in superfluid 4He

    NASA Astrophysics Data System (ADS)

    Mateo, David; Eloranta, Jussi; Williams, Gary A.

    2015-02-01

    The interaction of a number of impurities (H2, Ag, Cu, Ag2, Cu2, Li, He3 + , He* (3S), He2∗ (3Σu), and e-) with quantized rectilinear vortex lines in superfluid 4He is calculated by using the Orsay-Trento density functional theory (DFT) method at 0 K. The Donnelly-Parks (DP) potential function binding ions to the vortex is combined with DFT data, yielding the impurity radius as well as the vortex line core parameter. The vortex core parameter at 0 K (0.74 Å) obtained either directly from the vortex line geometry or through the DP potential fitting is smaller than previously suggested but is compatible with the value obtained from re-analysis of the Rayfield-Reif experiment. All of the impurities have significantly higher binding energies to vortex lines below 1 K than the available thermal energy, where the thermally assisted escape process becomes exponentially negligible. Even at higher temperatures 1.5-2.0 K, the trapping times for larger metal clusters are sufficiently long that the previously observed metal nanowire assembly in superfluid helium can take place at vortex lines. The binding energy of the electron bubble is predicted to decrease as a function of both temperature and pressure, which allows adjusting the trap depth for either permanent trapping or to allow thermally assisted escape. Finally, a new scheme for determining the trapping of impurities on vortex lines by optical absorption spectroscopy is outlined and demonstrated for He*.

  16. Interaction of Ions, Atoms and Small Molecules with Quantized Vortex Lines in Superfluid 4He

    NASA Astrophysics Data System (ADS)

    Eloranta, Jussi; Matteo, David; Williams, Gary

    2015-03-01

    The interaction of a number of impurities (H2, Ag, Cu, Ag2, Cu2, Li, He3+,He* (3 S), He2*(3Σu) and e-) with quantized rectilinear vortex lines in superfluid 4He is calculated using density functional methods at 0 K. The technique yields the impurity radius as well as the vortex line core parameter. The core parameter at 0 K (0.74 Å) obtained either directly from the vortex line geometry or from the trapping potential fitting is smaller than previously suggested but is compatible with a re-analysis of the Rayfield-Reif experiment. All of the impurities have significant binding energies to the vortex lines below 1 K where the thermally assisted escape process becomes very inefficient. Even at higher temperatures the trapping times, especially for larger clusters, are sufficiently long that the observed metal nanowire assembly in superfluid helium can take place at vortex lines. The binding energy of the electron bubble is predicted to decrease as a function of both temperature and pressure, which allows adjusting the trap depth for either permanent trapping or thermally assisted escape. A new scheme for determining the trapping of impurities on vortex lines by optical absorption spectroscopy is outlined and demonstrated for He*. Work supported by the NSF, Grants CHE-1262306 and DMR-1205734, and the Interdisciplinary Research Institute for the Sciences.

  17. One-Dimensional Liquid ^{4}He: Dynamical Properties beyond Luttinger-Liquid Theory.

    PubMed

    Bertaina, G; Motta, M; Rossi, M; Vitali, E; Galli, D E

    2016-04-01

    We compute the zero-temperature dynamical structure factor of one-dimensional liquid ^{4}He by means of state-of-the-art quantum Monte Carlo and analytic continuation techniques. By increasing the density, the dynamical structure factor reveals a transition from a highly compressible critical liquid to a quasisolid regime. In the low-energy limit, the dynamical structure factor can be described by the quantum hydrodynamic Luttinger-liquid theory, with a Luttinger parameter spanning all possible values by increasing the density. At higher energies, our approach provides quantitative results beyond the Luttinger-liquid theory. In particular, as the density increases, the interplay between dimensionality and interaction makes the dynamical structure factor manifest a pseudo-particle-hole continuum typical of fermionic systems. At the low-energy boundary of such a region and moderate densities, we find consistency, within statistical uncertainties, with predictions of a power-law structure by the recently developed nonlinear Luttinger-liquid theory. In the quasisolid regime, we observe a novel behavior at intermediate momenta, which can be described by new analytical relations that we derive for the hard-rods model.

  18. Biological concentration of /sup 3/H

    SciTech Connect

    Moghissi, A.A.; Bretthauer, E.W.; Patzer, R.G.

    1987-10-01

    In a three-year study, the possible biological concentration of /sup 3/H in rabbits was investigated. Tritiated water was used to grow alfalfa that was used exclusively as feed for the rabbits. Feed and water were kept at a constant /sup 3/H-to-/sup 1/H ratio. The foundation group consisted of 18 female rabbits maintained on a /sup 3/H diet for 2 wk before mating. The subsequent generations were maintained with tritiated water and feed. At appropriate intervals, animals were sacrificed and selected tissues were analyzed for /sup 3/H. The specific activity of /sup 3/H in aqueous and organic fractions of tissues of all the animals remained essentially equal to that in the original water and feed. Results of this experiment indicate that under the steady-state equilibrium conditions of the experiment, no preferential concentration of /sup 3/H in animals occurred.

  19. Electron screening and stellar rates in the {sup 3}He({sup 3}He,2p){sup 4}He and {sup 3}He(d,p){sup 4}He fusion reactions

    SciTech Connect

    Messahel, L.; Ouichaoui, S.; Belhout, A.; Fouka, M.; Trabelsi, A.

    2008-05-12

    The astrophysical S(E) factor experimental data available over the energy region E (C.M.)<1.0 MeV for the {sup 3}He({sup 3}He,2p){sup 4}He and {sup 3}He(d,p){sup 4}He fusion reactions are analyzed using a polynomial expression and the R-Matrix formalism, respectively. The reaction thermonuclear rates for bare nuclei are determined and compared to previous ones after a precise assessment of the electron screening factors. New level parameter values are deduced for the {sup 5}Li nucleus.

  20. 190Pt-4He age of PGE ores in the Alkaline-Ultramafic Kondyor Massif (Khabarovsk District, Russia)

    NASA Astrophysics Data System (ADS)

    Mochalov, A. G.; Yakubovich, O. V.; Bortnikov, N. S.

    2016-08-01

    A new 190Pt-4He method for dating isoferroplatinum has been developed at the Institute of Precambrian Geology and Geochronology, Russian Academy of Sciences. Here we publish the first results of dating of isoferroplatinum from the main mineralogical and geochemical types of PGE mineralization in dunite. The obtained 190Pt-4He age of isoferroplatinum is 129 ± 6 Ma. The gained 190Pt-4He age of isoferroplatinum specimens of different genesis (magmatic, fluid-metamorphogenic, and metasomatic) from the Kondyor Massif indicates that the PGM mineralization took place synchronously and successively with evolution of primarily picrite, followed by subalkaline and alkaline melts of the Mesozoic tectonic-magmatic activation of the Aldan Shield.

  1. Suppression of Freezing and Emergence of a Novel Ordered State in 4He Confined in a Nano - porous Material

    SciTech Connect

    Yamamoto, K.; Shibayama, Y.; Shirahama, K.

    2006-09-07

    Confinement of 4He in a porous material with nanometer - size pores suppresses both the freezing and superfluidity. In our previous investigation of superfluid density of 4He confined in a porous Gelsil glass which has pores of 2.5 nm in diameter, it was demonstrated that the superfluidity is greatly suppressed by pressurization. In order to explore the overall P - T phase diagram, we study the liquid - solid coexistence line. The freezing pressure is elevated up to about 3.4 MPa and independent of temperature below 1.3 K. Along with the previous measurement of superfluid density these features indicate that a nonsuperfluid phase exists next to the solid phase. The flat freezing curve indicates that this nonsuperfluid phase has small entropy as well as that of solid. Therefore the nonsuperfluid phase is possibly a novel ordered state, in which the global phase coherence is destroyed by strong correlation between 4He atoms and/or by random potential.

  2. Bare-nucleus astrophysical factor of the 3He(d,p)4He reaction via the ``Trojan horse'' method

    NASA Astrophysics Data System (ADS)

    La Cognata, M.; Spitaleri, C.; Tumino, A.; Typel, S.; Cherubini, S.; Lamia, L.; Musumarra, A.; Pizzone, R. G.; Rinollo, A.; Rolfs, C.; Romano, S.; Schürmann, D.; Strieder, F.

    2005-12-01

    The 3He(d,p)4He reaction has been studied from Ec.m.=600 keV down to astrophysical energies by means of the “Trojan horse” method using the 6Li(3He,pα)4He three-body reaction at Elab=5 and 6 MeV. Coincidence spectra were measured in kinematic conditions favoring the quasifree 3He+2H process. The bare astrophysical factor Sb(E) for the 3He(d,p)4He reaction was extracted from the three-body cross section in the modified plane-wave Born approximation. Comparison with the Sb extrapolation from the free two-body data is presented. The independent estimate of the screening potential as obtained with the present work seems to confirm the theoretical adiabatic limit.

  3. The nature of superfluidity and Bose-Einstein condensation: From liquid 4He to dilute ultracold atomic gases (Review Article)

    NASA Astrophysics Data System (ADS)

    Vilchynskyy, S. I.; Yakimenko, A. I.; Isaieva, K. O.; Chumachenko, A. V.

    2013-09-01

    We present a brief overview of crucial historical stages in creation of superfluidity theory and of the current state of the microscopic theory of superfluid 4He. We pay special attention to the role of Bose-Einstein condensates (BECs) in understanding of physical mechanisms of superfluidity and identification of quantum mechanical structure of 4He superfluid component below λ-point, in particular—the possibility that at least two types of condensates may appear and coexist simultaneously in superfluid 4He. In this context we discuss the properties of the binary mixtures of BECs and types of excitations, which may appear due to intercomponent interaction in such binary mixtures of condensates. We also discuss current status of investigations of persistent currents in toroidal optical traps and present an outlook of our recent findings on this subject.

  4. Interaction of ions, atoms, and small molecules with quantized vortex lines in superfluid {sup 4}He

    SciTech Connect

    Mateo, David; Eloranta, Jussi; Williams, Gary A.

    2015-02-14

    The interaction of a number of impurities (H{sub 2}, Ag, Cu, Ag{sub 2}, Cu{sub 2}, Li, He{sub 3}{sup +}, He{sup *} ({sup 3}S), He{sub 2}{sup ∗} ({sup 3}Σ{sub u}), and e{sup −}) with quantized rectilinear vortex lines in superfluid {sup 4}He is calculated by using the Orsay-Trento density functional theory (DFT) method at 0 K. The Donnelly-Parks (DP) potential function binding ions to the vortex is combined with DFT data, yielding the impurity radius as well as the vortex line core parameter. The vortex core parameter at 0 K (0.74 Å) obtained either directly from the vortex line geometry or through the DP potential fitting is smaller than previously suggested but is compatible with the value obtained from re-analysis of the Rayfield-Reif experiment. All of the impurities have significantly higher binding energies to vortex lines below 1 K than the available thermal energy, where the thermally assisted escape process becomes exponentially negligible. Even at higher temperatures 1.5-2.0 K, the trapping times for larger metal clusters are sufficiently long that the previously observed metal nanowire assembly in superfluid helium can take place at vortex lines. The binding energy of the electron bubble is predicted to decrease as a function of both temperature and pressure, which allows adjusting the trap depth for either permanent trapping or to allow thermally assisted escape. Finally, a new scheme for determining the trapping of impurities on vortex lines by optical absorption spectroscopy is outlined and demonstrated for He{sup *}.

  5. Second-sound studies of coflow and counterflow of superfluid {sup 4}He in channels

    SciTech Connect

    Varga, Emil; Skrbek, L.; Babuin, Simone

    2015-06-15

    We report a comprehensive study of turbulent superfluid {sup 4}He flow through a channel of square cross section. We study for the first time two distinct flow configurations with the same apparatus: coflow (normal and superfluid components move in the same direction), and counterflow (normal and superfluid components move in opposite directions). We realise also a variation of counterflow with the same relative velocity, but where the superfluid component moves while there is no net flow of the normal component through the channel, i.e., pure superflow. We use the second-sound attenuation technique to measure the density of quantised vortex lines in the temperature range 1.2 K ≲ T ≲ T{sub λ} ≈ 2.18 K and for flow velocities from about 1 mm/s up to almost 1 m/s in fully developed turbulence. We find that both the steady-state and temporal decay of the turbulence significantly differ in the three flow configurations, yielding an interesting insight into two-fluid hydrodynamics. In both pure superflow and counterflow, the same scaling of vortex line density with counterflow velocity is observed, L∝V{sub cf}{sup 2}, with a pronounced temperature dependence; in coflow instead, the vortex line density scales with velocity as L ∝ V{sup 3/2} and is temperature independent; we provide theoretical explanations for these observations. Further, we develop a new promising technique to use different second-sound resonant modes to probe the spatial distribution of quantised vortices in the direction perpendicular to the flow. Preliminary measurements indicate that coflow is less homogeneous than counterflow/superflow, with a denser concentration of vortices between the centre of the channel and its walls.

  6. Helium isotopes in early Iceland plume picrites: Constraints on the composition of high 3He/ 4He mantle

    NASA Astrophysics Data System (ADS)

    Starkey, Natalie A.; Stuart, Finlay M.; Ellam, Robert M.; Fitton, J. Godfrey; Basu, Sudeshna; Larsen, Lotte M.

    2009-01-01

    A detailed study of the geochemistry of a new suite of early Iceland plume picrites shows that extremely high 3He/ 4He ratios (up to 50 Ra) are found in picrites from Baffin Island and West Greenland. High 3He/ 4He picrites display a wide range in 87Sr/ 86Sr (0.70288-0.70403), 143Nd/ 144Nd (0.51288-0.51308) and incompatible trace element ratios (e.g. La/Sm n = 0.5-1.6). These overlap the complete range of compositions of mid-ocean ridge basalts and most northern hemisphere ocean island basalts, including Iceland. Crustal contamination modelling in which high-grade Proterozoic crustal basement rocks for the region are mixed with a depleted parent cannot account for the trend displayed by the Baffin Island and West Greenland picrites. This rules out the possibility that the incompatible trace element, Sr and Nd isotope range of the high 3He/ 4He picrites is due to crustal contamination. The compositional range at high 3He/ 4He is also inconsistent with derivation from a primordial-He-rich reservoir that is a residue of ancient mantle depletion. This implies that the composition of the high 3He/ 4He mantle cannot be determined simply by extrapolating ocean island basalt He-Sr-Nd-Pb-Os isotope data. The apparent decoupling of He from trace element and lithophile radiogenic isotope tracers is difficult to attain by simple mixing of a high-[He], high 3He/ 4He reservoir with various depleted and enriched He-poor mantle reservoirs. The possibility that primordial He has diffused into a reservoir with a composition typical of convecting upper mantle cannot be ruled out. If so, the process must have occurred after the development of existing mantle heterogeneity, and requires the existence of a deep, primordial He-rich reservoir.

  7. Pole approximation validation in the study of the {sup 6}Li(d,{alpha}){sup 4}He reaction

    SciTech Connect

    Pizzone, R. G.; Kiss, G. G.; Spitaleri, C.; Lamia, L.; Cherubini, S.; La Cognata, M.; Puglia, S. M. R.; Rapisarda, G. G.; Romano, S.; Sergi, M. L.; Burjan, V.; Hons, Z.; Kroha, V.; Mrazek, J.; Piskor, S.; Li, C.; Tumino, A.

    2010-11-24

    The Trojan Horse Method (THM) was applied to the {sup 3}He+{sup 6}Li interaction in order to investigate the quasi-free {sup 6}Li(d,{alpha}){sup 4}He reaction. The experiment was performed at 17 MeV at the Cyclotron Institute of the Czech Academy of Science. The extracted {sup 6}Li(d,{alpha}){sup 4}He quasi-free cross-section was compared with the behavior of direct data. A good agreement between data sets shows up throughout the energy range investigated, providing a very important validity test of the pole approximation for the THM above the Coulomb barrier.

  8. Mass Flux Stability in the Presence of Temperature Excursions and Perturbations in Solid ^3He-^4He Mixtures

    NASA Astrophysics Data System (ADS)

    Vekhov, Ye.; Hallock, R. B.

    2016-11-01

    The DC superfluid ^4He mass flux through a cell filled with solid ^4He diluted by ppm amounts of ^3He is susceptible to flux changes when perturbations of the solid sample are imposed. We report on the details of the reproducibility of the flux following excursions in temperature and cryostat helium transfer-induced apparatus vibration, particularly including excursions to temperatures above which the flux is immeasurably small. And we report on behavior following an annealing, partial melting, and re-freezing of the sample at temperatures and pressures close to and on the melting curve.

  9. Geometrical symmetries of nuclear systems: {{ D }}_{3h} and {{ T }}_{d} symmetries in light nuclei

    NASA Astrophysics Data System (ADS)

    Bijker, Roelof

    2016-07-01

    The role of discrete (or point-group) symmetries in α-cluster nuclei is discussed in the framework of the algebraic cluster model which describes the relative motion of the α-particles. Particular attention is paid to the discrete symmetry of the geometric arrangement of the α-particles, and the consequences for the structure of the corresponding rotational bands. The method is applied to study cluster states in the nuclei 12C and 16O. The observed level sequences can be understood in a simple way as a consequence of the underlying discrete symmetry that characterizes the geometrical configuration of the α-particles, i.e. an equilateral triangle with {{ D }}3h symmetry for 12C, and a tetrahedron with {{ T }}d symmetry for 16O. The structure of rotational bands provides a fingerprint of the underlying geometrical configuration of α-particles.

  10. Temperature dependence of S(Q,ω) in liquid 4He under pressure

    NASA Astrophysics Data System (ADS)

    Talbot, E. F.; Glyde, H. R.; Stirling, W. G.; Svensson, E. C.

    1988-12-01

    The temperature dependence of the dynamic form factor, S(Q,ω), of liquid 4He at p=20 bars has been determined by inelastic neutron scattering measurements. Two wave vectors, Q=1.13 Å-1 and Q=2.03 Å-1, corresponding to the maxon and roton regions of the phonon-roton dispersion curve, were studied over a wide range of energy transfer, ħω. Based on previous data at SVP, Woods and Svensson proposed that S(Q,ω) could be represented as a sum of two components, one proportional to the superfluid density, ρS(T), and one proportional to the normal density ρN(T). The component proportional to ρS(T) contained the sharp one-phonon peak which vanished at T=Tλ. The aim here is, firstly, to present data on the temperature dependence of S(Q,ω) at 20 bars and, secondly, to explore whether or not the Woods-Svensson decomposition of S(Q,ω) holds at higher pressure. At 20 bars and for the Q values investigated here, we find that the sharp peak of S(Q,ω) does indeed decrease rapidly in intensity as T increases and the corresponding excitation either vanishes or changes abruptly in character at Tλ. The sharp nature of the one-phonon peak Tλ does therefore appear to be associated with superfluidity or a Bose condensate at these Q values. However, the weight of the one-phonon peak does not scale as ρS(T) and subtracting a contribution proportional to ρN(T) from S(Q,ω) leads to negative values of the superfluid component of S(Q,ω) at low ω. Thus S(Q,ω) at 20 bars does not naturally separate into a part proportional to ρS and one proportional to ρN. We also explore the consequences of a simple subtraction of the multiphonon component, assumed temperature independent, as an alternative method of extracting one-phonon parameters from the total scattering intensity. The values of the one-phonon properties such as the frequency and the lifetime obtained by the simple multiphonon subtraction method also show a marked change at Tλ.

  11. Spectroscopic information of 6Li from elastic scattering of deuterons, 3He and 4He by 6Li

    NASA Astrophysics Data System (ADS)

    Amar, A.

    2014-07-01

    The elastic scattering of deuterons, 3He and 4He on 6Li at different incident energies have been analyzed in the framework of the optical model (OM) using ECIS88 as well as SPI GENOA codes. The optical potential parameters were extracted in the phenomenological treatment. A good agreement between theoretical and experimental differential cross-sections was obtained in whole angular range. Parameters for real part of potential have been also calculated microscopically with double-folding model for the d, 3He and 4He scattering, respectively, using DFPOT code. The elastic transfer mechanism has been studied by coupled reaction channel (CRC) method using FRESCO code. Spectroscopic amplitudes of 6Li ≡ t + 3He and 6Li ≡ α + d configurations have been extracted from d, 3He and 4He scattering on 6Li at wide energy range. A comparison between spectroscopic amplitudes obtained from deuteron and α elastically scattering from 6Li has been made. The extracted spectroscopic amplitudes of 6Li ≡ 4He + d(SF = SA2) from 6Li(d, 6Li)d and 6Li(α, 6Li)α are not the same as expected theoretically.

  12. Incorporating 3-D parent nuclide zonation for apatite 4He/3He thermochronometry: An example from the Appalachian Mountains

    NASA Astrophysics Data System (ADS)

    Fox, Matthew; McKeon, Ryan E.; Shuster, David L.

    2014-11-01

    ability to constrain km-scale exhumation with apatite 4He/3He thermochronometry is well established and the technique has been applied to a range of tectonic and geomorphic problems. However, multiple sources of uncertainty in specific crystal characteristics limit the applicability of the method, especially when geologic problems require identifying small perturbations in a cooling path. Here we present new 4He/3He thermochronometric data from the Appalachian Mountains, which indicate significant parent nuclide zonation in an apatite crystal. Using LA-ICPMS measurements of U and Th in the same crystal, we design a 3-D model of the crystal to explore the effects of intracrystal variability in radiation damage accumulation. We describe a numerical approach to solve the 3-D production-diffusion equation. Using our numerical model and a previously determined time temperature path for this part of the Appalachians, we find excellent agreement between predicted and observed 4He/3He spectra. Our results confirm this time-temperature path and highlight that for complex U and Th zonation patterns, 3-D numerical models are required to infer an accurate time-temperature history. In addition, our results provide independent and novel evidence for a radiation damage control on diffusivity. The ability to exploit intracrystal differences in 4He diffusivity [i.e., temperature sensitivity) greatly increases the potential to infer complex thermal histories.

  13. 4He in Modern Cape Verde Corals: A High-Resolution Proxy Record of N. African Climate

    NASA Astrophysics Data System (ADS)

    Mukhopadhyay, S.; Kreycik, P.; Schrag, D. P.

    2005-12-01

    Mineral dust from arid and semi arid regions is an important component of climatic processes. The amount of dust emitted off continents is intimately linked with precipitation, which may itself be linked to atmospheric circulation driven by oceanic sea surface temperatures. Hence, reconstructing dust fluxes off continents with sub-decadal resolution can provide us with fundamental insights into feedbacks in the climate system. Unfortunately, such high-resolution dust flux records prior to the establishment of the Barbados dust sampling station are largely lacking. Here we show that 4He concentrations in annual bands in corals provides a high-resolution, reliable, and robust proxy record of dust flux from continents. Some traces phases in dust, such as zircons, are rich in U and Th and thus have extremely high concentrations of 4He. As some fraction of the dust settles out of the atmosphere and through the water column, corals incorporate the dust in their skeletons through filter feeding. Since the alpha stopping distance is greater than the particle size of wind blown dust, the mineral grains will not accumulate radiogenic helium after the dust is incorporated into the corals. We have measured the 4He concentration in annual bands dating back to 1960's in a modern coral that was collected in 1996 off the island of Sal, part of the Cape Verde archipelago. The coral is therefore, situated close to, and directly west of the dust source in the Sudano-Sahel region of the African continent. The 4He record from the coral shows remarkable similarity with the record from the Barbados dust sampling station. There is a continuous increase in 4He baseline values by a factor of two from the mid 1960's to the early 1990's as well as two pronounced peaks in the early 1970's and mid 1980's associated with severe drought in the Sudano-Sahel region. Our proxy record from the Cape Verde Island demonstrates that 4He concentrations in corals can be used reliably to reconstruct dust

  14. The helium flux from the continents and ubiquity of low-3He/4He recycled crust and lithosphere

    NASA Astrophysics Data System (ADS)

    Day, James M. D.; Barry, Peter H.; Hilton, David R.; Burgess, Ray; Pearson, D. Graham; Taylor, Lawrence A.

    2015-03-01

    New helium isotope and trace-element abundance data are reported for pyroxenites and eclogites from South Africa, Siberia, and the Beni Bousera Massif, Morocco that are widely interpreted to form from recycled oceanic crustal protoliths. The first He isotope data are also presented for Archaean peridotites from the Kaapvaal (South Africa), Slave (Canada), and Siberian cratons, along with recently emplaced off-craton peridotite xenoliths from Kilbourne Hole, San Carlos (USA) and Vitim (Siberia), to complement existing 3He/4He values obtained for continental and oceanic peridotites. Helium isotope compositions of peridotite xenoliths vary from 7.3 to 9.6 RA in recently (<10 kyr) emplaced xenoliths, to 0.05 RA in olivine from cratonic peridotite xenoliths of the 1179 Ma Premier kimberlite, South Africa. The helium isotope compositions of the peridotites can be explained through progressive sampling of 4He produced from radiogenic decay of U and Th in the mineral lattice in the older emplaced peridotite xenoliths. Ingrowth of 4He is consistent with generally higher 4He concentrations measured in olivine from older emplaced peridotite xenoliths relative to those from younger peridotite xenoliths. Collectively, the new data are consistent with pervasive open-system behaviour of He in peridotite xenoliths from cratons, mobile belts and tectonically-active regions. However, there is probable bias in the estimate of the helium isotope composition of the continental lithospheric mantle (6.1 ± 2.1 RA), since previously published databases were largely derived from peridotite xenoliths from non-cratonic lithosphere, or phenocrysts/xenocrysts obtained within continental intraplate alkaline volcanics that contain a contribution from asthenospheric sources. Using the new He isotope data for cratonic peridotites and assuming that significant portions (>50%) of the Archaean and Proterozoic continental lithospheric mantle are stable and unaffected by melt or fluid infiltration on

  15. Enhancing the branching ratios in the dissociation channels for O(16)O(16)O(18) molecule by designing optimum laser pulses: A study using stochastic optimization.

    PubMed

    Talukder, Srijeeta; Sen, Shrabani; Shandilya, Bhavesh K; Sharma, Rahul; Chaudhury, Pinaki; Adhikari, Satrajit

    2015-10-14

    We propose a strategy of using a stochastic optimization technique, namely, simulated annealing to design optimum laser pulses (both IR and UV) to achieve greater fluxes along the two dissociating channels (O(18) + O(16)O(16) and O(16) + O(16)O(18)) in O(16)O(16)O(18) molecule. We show that the integrated fluxes obtained along the targeted dissociating channel is larger with the optimized pulse than with the unoptimized one. The flux ratios are also more impressive with the optimized pulse than with the unoptimized one. We also look at the evolution contours of the wavefunctions along the two channels with time after the actions of both the IR and UV pulses and compare the profiles for unoptimized (initial) and optimized fields for better understanding the results that we achieve. We also report the pulse parameters obtained as well as the final shapes they take. PMID:26472365

  16. Communication: A combined periodic density functional and incremental wave-function-based approach for the dispersion-accounting time-resolved dynamics of {sup 4}He nanodroplets on surfaces: {sup 4}He/graphene

    SciTech Connect

    Lara-Castells, María Pilar de; Stoll, Hermann; Civalleri, Bartolomeo; Causà, Mauro; Voloshina, Elena; Mitrushchenkov, Alexander O.; Pi, Martí

    2014-10-21

    In this work we propose a general strategy to calculate accurate He–surface interaction potentials. It extends the dispersionless density functional approach recently developed by Pernal et al. [Phys. Rev. Lett. 103, 263201 (2009)] to adsorbate-surface interactions by including periodic boundary conditions. We also introduce a scheme to parametrize the dispersion interaction by calculating two- and three-body dispersion terms at coupled cluster singles and doubles and perturbative triples (CCSD(T)) level via the method of increments [H. Stoll, J. Chem. Phys. 97, 8449 (1992)]. The performance of the composite approach is tested on {sup 4}He/graphene by determining the energies of the low-lying selective adsorption states, finding an excellent agreement with the best available theoretical data. Second, the capability of the approach to describe dispersionless correlation effects realistically is used to extract dispersion effects in time-dependent density functional simulations on the collision of {sup 4}He droplets with a single graphene sheet. It is found that dispersion effects play a key role in the fast spreading of the {sup 4}He nanodroplet, the evaporation-like process of helium atoms, and the formation of solid-like helium structures. These characteristics are expected to be quite general and highly relevant to explain experimental measurements with the newly developed helium droplet mediated deposition technique.

  17. A HETEROGENEOUS CHEMICAL ORIGIN FOR THE {sup 16}O-ENRICHED AND {sup 16}O-DEPLETED RESERVOIRS OF THE EARLY SOLAR SYSTEM

    SciTech Connect

    Dominguez, Gerardo

    2010-04-10

    The oldest solids formed in the solar system, calcium-aluminum inclusions, are {sup 16}O-enriched compared to chondrules, asteroids, Earth, and Mars. Based on the preliminary measurements of the solar wind by Genesis, the Sun also appears to be {sup 16}O-enriched. This distribution of oxygen isotopes in the solar system cannot be reconciled via conventional mass-dependent isotopic fractionation processes and instead require the existence and/or production of distinct {sup 16}O-enriched and {sup 16}O-depleted reservoirs in the early solar system. The origin of these distinct reservoirs is unknown, although several mechanisms have been proposed to date including the following: (1) the injection of pure {sup 16}O by a supernova into the protoplanetary disk or parent molecular cloud, (2) self-shielding of CO in the parent molecular cloud or protoplanetary disk, (3) symmetry-dependent chemical fractionation processes in the protoplanetary disk, and (4) Galactic chemical evolution. While some of these proposals have been ruled out, the validity of others is still open. Here I propose that the {sup 16}O-enriched and {sup 16}O-depleted reservoirs present in the early solar system originated in the parent molecular cloud via the heterogeneous chemical processes that form H{sub 2}O, a significant oxygen reservoir, on the surface of interstellar (IS) dust grains in dense molecular clouds, the astrophysical setting where star formation is observed to occur. As a consequence, this model predicts that molecular cloud H{sub 2}O and possibly other IS solids inherited from the molecular cloud were depleted in {sup 16}O compared to the bulk gas-phase O present, thus providing distinct {sup 16}O reservoirs at the earliest stages of planetary formation.

  18. Laser spectroscopy of thulium atoms implanted in liquid and solid 4He

    NASA Astrophysics Data System (ADS)

    Ishikawa, Kiyoshi; Hatakeyama, Atsushi; Koichi, Gosyono-O.; Wada, Shigeaki; Takahashi, Yoshiro; Yabuzaki, Tsutomu

    1997-07-01

    The excitation, emission spectra, and decay curves of the emission intensity of thulium atoms implanted in liquid and solid helium were observed in the presence and absence of an external magnetic field. The observed narrow line (width ~0.1 nm) of the excitation spectrum at 590.60 nm is assigned as a zero-phonon transition from the electronic ground state 4f13(2Fo7/2)6s2, which indicates that the transition between the inner shells is weakly perturbed by surrounding helium atoms. The pressure dependence of the emission wavelength suggests that the symmetry of helium atoms distributed around a thulium atom in the solid phase is similar to that in the liquid phase. The emission intensity was stable and large in the solid phase since thulium atoms were trapped at a density of 1010-1011 atoms/cm3. The lifetime of the excited state was measured to be 7.09+/-0.04 μs, which was longer than that of the 4f12(3H6)5d5/26s2 (6,5/2)7/2 state of free thulium atoms. The excited state is expected to be a mixed state of the 4f125d6s2 and 4f136s6p configurations. The metastable state 4f13(2Fo5/2)6s2 is populated by a radiative transition from this excited state and relaxes to the ground state through a magnetic dipole transition. The lifetime of the metastable state of a neutral thulium atom was measured to be 75+/-3 ms.

  19. Theoretical estimates of the critical exponents of the superfluid transition in {sup 4}He by lattice methods

    SciTech Connect

    Campostrini, Massimo; Hasenbusch, Martin; Vicari, Ettore; Pelissetto, Andrea

    2006-10-01

    We improve the theoretical estimates of the critical exponents for the three-dimensional XY universality class that apply to the superfluid transition in {sup 4}He along the {lambda} line of its phase diagram. We obtain the estimates {alpha}=-0.0151(3), {nu}=0.6717(1), {eta}=0.0381(2), {gamma}=1.3178(2), {beta}=0.3486(1), and {delta}=4.780(1). Our results are obtained by finite-size scaling analyses of high-statistics Monte Carlo simulations up to lattice size L=128 and resummations of 22nd-order high-temperature expansions of two improved models with suppressed leading scaling corrections. We note that our result for the specific-heat exponent {alpha} disagrees with the most recent experimental estimate {alpha}=-0.0127(3) at the superfluid transition of {sup 4}He in a microgravity environment.

  20. STUDY OP THE 12C(α, γ)16O REACTION BY BREAKUP OF A 16O -BEAM AT 100 MeV/A

    NASA Astrophysics Data System (ADS)

    Tatischeff, V.; Kiener, J.; Aguer, P.; Angulo-Perez, C.; Bogaert, G.; Coc, A.; Disdier, D.; Ichihara, T.; Kraus, L.; Lefebvre, A.; Linck, I.; Mittig, W.; Motobayashi, T.; Oliveira, F.; Roussel-Chomaz, P.; Stephan, C.; Thibaud, J. P.

    We present some preliminary calculations on cross sections for the breakup of 16O around 100 MeV/A with emphasis on the effect of nuclear breakup on the angular distributions. Underlying the results of these calculations, the possibilities and problems of extracting the astrophysical S-factor for the 12C(α, γ)16O reaction at very low energies are discussed. Some considerations on the experimental conditions for a 16O breakup experiment aiming at this astrophysical information, are given.

  1. Are high 3He/4He ratios in oceanic basalts an indicator of deep-mantle plume components?

    USGS Publications Warehouse

    Meibom, A.; Anderson, D.L.; Sleep, N.H.; Frei, R.; Chamberlain, C.P.; Hren, M.T.; Wooden, J.L.

    2003-01-01

    The existence of a primordial, undegassed lower mantle reservoir characterized by high concentration of 3He and high 3He/4He ratios is a cornerstone assumption in modern geochemistry. It has become standard practice to interpret high 3He/4He ratios in oceanic basalts as a signature of deep-rooted plumes. The unfiltered He isotope data set for oceanic spreading centers displays a wide, nearly Gaussian, distribution qualitatively similar to the Os isotope (187Os/188 Os) distribution of mantle-derived Os-rich alloys. We propose that both distributions are produced by shallow mantle processes involving mixing between different proportions of recycled, variably aged radiogenic and unradiogenic domains under varying degrees of partial melting. In the case of the Re-Os isotopic system, radiogenic mid-ocean ridge basalt (MORB)-rich and unradiogenic (depleted mantle residue) endmembers are constantly produced during partial melting events. In the case of the (U+Th)-He isotope system, effective capture of He-rich bubbles during growth of phenocryst olivine in crystallizing magma chambers provides one mechanism for 'freezing in' unradiogenic (i.e. high 3He/4He) He isotope ratios, while the higher than chondritic (U+Th)/He elemental ratio in the evolving and partially degassed MORB melt provides the radiogenic (i.e. low 3He/4He) endmember. If this scenario is correct, the use of He isotopic signatures as a fingerprint of plume components in oceanic basalts is not justified. Published by Elsevier Science B.V.

  2. Production of {sup 4}He, {sup 3}He, and tritium from Be irradiated in FFTF-MOTA-2B

    SciTech Connect

    Greenwood, L.R.

    1998-03-01

    The production of {sup 4}He, {sup 3}He, and tritium has been calculated for beryllium irradiated in the Materials Open Test Assembly (MOTA)-2B experiment in the Fast Flux Test Facility (FFTF). Reaction rates were based on adjusted neutron spectra determined from reactor dosimetry measurements at seven different elevations in the irradiation assembly. Equations are given so that gas production, dpa, and neutron fluences can be calculated for any specific elevation in the MOTA-2B assembly.

  3. Motion of a helical vortex filament in superfluid 4He under the extrinsic form of the local induction approximation

    NASA Astrophysics Data System (ADS)

    Van Gorder, Robert A.

    2013-08-01

    Very recently, Shivamoggi ["Vortex motion in superfluid 4He: Reformulation in the extrinsic vortex-filament coordinate space," Phys. Rev. B 84, 012506 (2011)], 10.1103/PhysRevB.84.012506 studied the extrinsic form of the local induction approximation (LIA) for the motion of a Kelvin wave on a vortex filament in superfluid 4He, and obtained some results in a cubic approximation. Presently, we study the motion of helical vortex filaments in superfluid 4He under the exact fully nonlinear LIA considered in potential form by Van Gorder ["Fully nonlinear local induction equation describing the motion of a vortex filament in superfluid 4He," J. Fluid Mech. 707, 585 (2012)], 10.1017/jfm.2012.308 and obtained from the Biot-Savart law through the equations of Hall and Vinen ["The rotation of liquid helium II. I. Experiments on the propagation of second sound in uniformly rotating helium II," Proc. R. Soc. London, Ser. A 238, 204 (1956)], 10.1098/rspa.1956.0214 including superfluid friction terms. Nonlinear dispersion relations governing the helical Kelvin wave on such a vortex filament are derived in exact form, from which we may exactly calculate the phase and group velocity of the Kelvin wave. With this, we classify the motion of a helical Kelvin wave on a vortex filament under the LIA. The dispersion relations and results, which follow are exact in nature, in contrast to most results in the literature, which are usually numerical approximations. As such, our results accurately capture the qualitative behavior of the Kelvin waves under the LIA. Extensions to other frameworks are discussed.

  4. The structure of mixed {sup 3}He-{sup 4}He droplets doped with OCS: A density functional approach

    SciTech Connect

    Leal, Antonio; Mateo, David; Pi, Martí; Barranco, Manuel; Navarro, Jesús

    2013-11-07

    We have investigated the structure and energetics of mixed {sup 3}He-{sup 4}He droplets doped with a carbonyl sulfide molecule within a density functional approach considering a small but finite temperature of 0.1 K. The molecule is treated as an external field to which the helium droplet is attached. The energetics and appearance of these droplets are discussed for selected numbers of helium atoms, identifying the first magic numbers of the fermionic component.

  5. Static and thermodynamic properties of low-density supercritical 4He-breakdown of the Feynman-Hibbs approximation.

    PubMed

    Kowalczyk, Piotr; Brualla, Lorenzo; Gauden, Piotr A; Terzyk, Artur P

    2009-10-28

    We study the applicability of the semiclassical Feynman and Hibbs (FH) (second-order or fourth-order) effective potentials to the description of the thermodynamic properties of quantum fluids at finite temperatures. First, we use path integral Monte Carlo (PIMC) simulations to estimate the thermodynamic/static properties of our model quantum fluid, i.e. low-density 4He at 10 K. With PIMC we obtain the experimental equation of state, the single-particle mean kinetic energy, the single-particle density matrix and the single-particle momentum distribution of this system at low densities. We show that our PIMC results are in full agreement with experimental data obtained with deep inelastic neutron scattering at high momentum transfers (D. Colognesi, C. Andreani, R. Senesi, Europhys. Lett., 2000, 50, 202). As expected, in this region of the 4He phase diagram, quantum effects modify the width of the single-particle momentum distribution but do not alter its Gaussian shape. Knowing the exact values of density, pressure and single-particle mean kinetic energy for our model quantum fluid, we investigate the limitations of the semiclassical FH effective potentials. We show that commonly used 'short-time' approximations to the high-temperature density matrix due to Feynman and Hibbs can only be applied in a very limited range of the 4He phase diagram. We found that FH effective potentials reproduce the experimental densities of 4He at 10 K for Lambda/a < 0.45 (Lambda = 2.73 A denotes the thermal de Broglie wavelength, a = rho(-1/3) is the mean nearest-neighbor distance in the fluid and rho denotes fluid density). Moreover, semiclassical FH effective potentials are able to correctly predict the single-particle mean kinetic energy of 4He at 10 K in a very limited range of fluid densities, i.e.Lambda/a < 0.17. We show that the ad hoc application of the semiclassical FH effective potentials for the calculation of the thermodynamic properties of dense liquid-like para

  6. Multichannel study of the {sup 13}C({alpha},n){sup 16}O and {sup 16}O(n,{gamma}){sup 17}O reactions

    SciTech Connect

    Dufour, M.; Descouvemont, P.

    2005-07-01

    The {sup 13}C({alpha},n){sup 16}O reaction is investigated in a microscopic two-cluster model with an effective interaction recently developed for transfer reactions. The wave functions are defined in the generator coordinate method. The basis includes all {sup 13}C+{alpha} and {sup 16}O+n channels with {sup 13}C and {sup 16}O described in the p shell. Particle-hole excitations in the sd shell are also taken into account in order to include the {sup 16}O(3{sup -})+n channel. The {sup 17}O spectroscopy is in good agreement with experiment. In particular, the width of the astrophysically relevant 1/2{sub 2}{sup +} state is well reproduced ({gamma}=121 keV as compared to the experimental value {gamma}=124{+-}12 keV). The calculation of the {sup 13}C({alpha},n){sup 16}O S factor shows the importance of the 3/2{sub 3}{sup +} resonance, and provides S(0.2 MeV)=2.1x10{sup 6} MeV b, slightly lower than the NACRE recommended value (2.5x10{sup 6} MeV b). The same model is applied to the {sup 16}O(n,{gamma}){sup 17}O radiative-capture reaction at thermal and astrophysical energies.

  7. Model-independent analysis of Airy structures in the {sup 16}O+{sup 12}C and {sup 16}O+{sup 16}O elastic scattering differential cross sections at 13-22 MeV/nucleon

    SciTech Connect

    Korda, V. Yu.; Molev, A. S.; Klepikov, V. F.; Korda, L. P.

    2009-02-15

    We present the results of the model-independent analysis of Airy structures in the {sup 16}O+{sup 12}C and {sup 16}O+{sup 16}O elastic scattering differential cross sections at 13-22 MeV/nucleon. The analysis has been performed with help of a procedure based on the application of the evolutionary algorithm, which enables us to extract the nuclear part of the scattering matrix S{sub N}(l) as a complex function of angular momentum directly from the scattering data. Contrary to the commonly used model approaches, our procedure gives the better fits and leads to the S{sub N}(l) representations defined by the moduli and the nuclear phases exhibiting smooth monotonic dependencies on l.

  8. High pressure line shapes of the Rb D1 and D2 lines for 4He and 3He collisions

    NASA Astrophysics Data System (ADS)

    Miller, Wooddy S.; Rice, Christopher A.; Hager, Gordon D.; Rotondaro, Mathew D.; Berriche, Hamid; Perram, Glen P.

    2016-11-01

    Line shapes for the Rb D1 (51/2 2S ↔ 51/2 2P) and D2 (51/2 2S ↔ 53/2 2P) transitions with 4He and 3He collisions at pressures of 500-15,000 Torr and temperatures of 333-533 K have been experimentally observed and compared to predictions from the Anderson-Talman theory. The ground X1/2 + 2Σ and excited A1/2 + 2Π, A3/2 2Π, and B1/2 + 2Σ potential energy surfaces required for the line shape predictions have been calculated using a one-electron pseudo-potential technique. The observed collision induced shift rates for 4He are dramatically higher for the D1 line, 4.60±0.12 MHz/Torr, than the D2 line, 0.20±0.14 MHz/Torr. The asymmetry is somewhat larger for the D1 line and has the same sign as the shifting rate. The 3He broadening rate for the D2 line is 4% larger than the 4He rate, and 14% higher for the D1 line, reflecting the higher relative speed. The calculated broadening rates are systematically larger than the observed rates by 1.1-3.2 MHz/Torr and agree within 14%. The primary focus of the current work is to characterize the high pressure line shapes, focusing on the non-Lorentzian features far from line center. In the far wing, the cross-section decreases by more than 4 orders of magnitude, with a broad, secondary maximum in the D2 line near 735 nm. The potentials do not require empirical modification to provide excellent quantitative agreement with the observations. The dipole moment variation and absorption Boltzmann factor is critical to obtaining strong agreement in the wings.

  9. Analysis of the scintillation mechanism in a pressurized {sup 4}He fast neutron detector using pulse shape fitting

    SciTech Connect

    Kelley, R.P. Ray, H.; Jordan, K.A.; Murer, D.

    2015-03-15

    An empirical investigation of the scintillation mechanism in a pressurized {sup 4}He gas fast neutron detector was conducted using pulse shape fitting. Scintillation signals from neutron interactions were measured and averaged to produce a single generic neutron pulse shape from both a {sup 252}Cf spontaneous fission source and a (d,d) neutron generator. An expression for light output over time was then developed by treating the decay of helium excited states in the same manner as the decay of radioactive isotopes. This pulse shape expression was fitted to the measured neutron pulse shape using a least-squares optimization algorithm, allowing an empirical analysis of the mechanism of scintillation inside the {sup 4}He detector. A further understanding of this mechanism in the {sup 4}He detector will advance the use of this system as a neutron spectrometer. For {sup 252}Cf neutrons, the triplet and singlet time constants were found to be 970 ns and 686 ns, respectively. For neutrons from the (d,d) generator, the time constants were found to be 884 ns and 636 ns. Differences were noted in the magnitude of these parameters compared to previously published data, however the general relationships were noted to be the same and checked with expected trends from theory. Of the excited helium states produced from a {sup 252}Cf neutron interaction, 76% were found to be born as triplet states, similar to the result from the neutron generator of 71%. The two sources yielded similar pulse shapes despite having very different neutron energy spectra, validating the robustness of the fits across various neutron energies.

  10. Astrophysical S factor for the 4He(3He,γ)7Be reaction at medium energies

    NASA Astrophysics Data System (ADS)

    Carmona-Gallardo, M.; Nara Singh, B. S.; Tengblad, O.; Hass, M.; Alcorta, M.; Borge, M. J. G.; Briz, J. A.; Cruz, C.; Cubero, M.; Domínguez-Reyes, R.; Fulton, B. R.; Fynbo, H.; Gordillo, N.; Haquin, G.; Nir-El, Y.; Kumar, V.; Maira, A.; McGrath, J.; Muñoz-Martín, A.; Perea, A.; Yungreis, Z.

    2012-02-01

    The astrophysical S factor for the 4He(3He,γ)7Be direct capture reaction plays a major role in the context of solar neutrino flux and primordial 7Li abundances that demand accurate information on the reaction. We report here our recent cross section measurements using the activation method in the region of ECM = 900-2800 keV, that aim to shed light on the discrepancies in the existing data and lead to a more accurate extrapolation of the S factor.

  11. Analysis of states in {sup 13}C populated in {sup 9}Be + {sup 4}He resonant scattering

    SciTech Connect

    Freer, M.; Ashwood, N. I.; Curtis, N.; Kokalova, Tz.; Wheldon, C.; Di Pietro, A.; Figuera, P.; Fisichella, M.; Scuderi, V.; Torresi, D.; Grassi, L.; Jelavic Malenica, D.; Koncul, M.; Mijatovic, T.; Prepolec, L.; Skukan, N.; Soic, N.; Szilner, S.; Tokic, V.; Milin, M.

    2011-09-15

    Measurements of {sup 9}Be + {alpha} resonant scattering have been performed using the thick-target approach with a {sup 4}He gas volume and a large-area silicon strip detector. {sup 9}Be beam energies in the range 12 to 21.4 MeV were used to measure the {sup 13}C excitation energy spectrum between 13.2 and 16.2 MeV. An R-matrix analysis has been performed to characterize the spins and widths of {sup 13}C resonances, some of which have been proposed to be associated with a 3{alpha}+n molecular band.

  12. Relationship between 3He/4He ratios and subduction of the Philippine Sea plate beneath southwest Japan

    NASA Astrophysics Data System (ADS)

    Umeda, Koji; Kusano, Tomohiro; Asamori, Koichi; McCrank, Glen F.

    2012-10-01

    Regional and local variations in mantle helium provide insight into the coupling of mantle-crust tectonics, and heat and/or mass transfer from the Earth's interior. In order to further elucidate the geographic distribution of3He/4He ratios in southwest Japan, the data from a total of 924 sites were compiled and synthesized. These include data from 48 additional hot spring and drinking water well sites on the northern Kyushu Island and in the northern Chugoku region. There appears to be good correlation between variations in helium isotope ratios and the geophysical evidence used to determine the configuration of the subducting Philippine Sea plate (PHS). Seismological studies reveal that the leading edge of the aseismic slab does not extend to the northern Chugoku region nor to the Osaka Bay area, where gas samples with significantly elevated 3He/4He ratios occur. This is consistent with a mantle-derived helium in these areas, from melts and/or mantle fluids ascribed to upwelling asthenosphere without being hindered by the descending PHS slab. In contrast, gas samples in the regions where the overriding crust comes into direct contact with the subducting PHS are dominated by radiogenic helium derived from the crust because of the absence of a mantle wedge, the most plausible source of mantle helium. Owing to the abrupt changes in the seismicity and focal mechanisms of intraplate earthquakes, the PHS is considered to have slab tears beneath the Kii Channel and/or the eastern Kii Peninsula oriented in a NW-SE direction. However, the lenear alignment of anomalously high3He/4He ratios does not appear to be NW-SE trending along the assumed slab tears but rather forms an broad, ENE-WSW trending zone between the tears where low-frequency events occur. The emanation of gas with elevated3He/4He ratios in the central peninsula can be explained by the upward mobilization of mantle volatiles derived from the mantle wedge above the PHS and/or transferred from the hydrated slab

  13. Assessing the use of 3H-3He dating to determine the subsurface transit time of cave drip waters.

    PubMed

    Kluge, Tobias; Wieser, Martin; Aeschbach-Hertig, Werner

    2010-09-01

    (3)H-(3)He measurements constitute a well-established method for the determination of the residence time of young groundwater. However, this method has rarely been applied to karstified aquifers and in particular to drip water in caves, despite the importance of the information which may be obtained. Besides the determination of transfer times of climate signals from the atmosphere through the epikarst to speleothems as climate archives, (3)H-(3)He together with Ne, Ar, Kr, Xe data may also help to give new insights into the local hydrogeology, e.g. the possible existence of a perched aquifer above a cave. In order to check the applicability of (3)H-(3)He dating to cave drips, we collected drip water samples from three adjacent caves in northwestern Germany during several campaigns. The noble gas data were evaluated by inverse modelling to obtain recharge temperature and excess air, supporting the calculation of the tritiogenic (3)He and hence the (3)H-(3)He age. Although atmospheric noble gases were often found to be close to equilibrium with the cave atmosphere, several drip water samples yielded an elevated (3)He/(4)He ratio, providing evidence for the accumulation of (3)He from the decay of (3)H. No significant contribution of radiogenic (4)He was found, corresponding to the low residence times mostly in the range of one to three years. Despite complications during sampling, conditions of a perched aquifer could be confirmed by replicate samples at one drip site. Here, the excess air indicator ΔNe was about 10 %, comparable to typical values found in aquifers in mid-latitudes. The mean (3)H-(3)He age of 2.1 years at this site presumably refers to the residence time in the perched aquifer and is lower than the entire transit time of 3.4 years estimated from the tritium data.

  14. Unified description of 6Li structure and deuterium-4He dynamics with chiral two- and three-nucleon forces

    DOE PAGES

    Hupin, Guillaume; Quaglioni, Sofia; Navratil, Petr

    2015-05-29

    Here, we provide a unified ab initio description of the 6Li ground state and elastic scattering of deuterium (d) on 4He (α) using two- and three-nucleon forces from chiral effective field theory. We analyze the influence of the three-nucleon force and reveal the role of continuum degrees of freedom in shaping the low-lying spectrum of 6Li. The calculation reproduces the empirical binding energy of 6Li, yielding an asymptotic D- to S-state ratio of the 6Li wave function in the d+α configuration of –0.027, in agreement with a determination from 6Li–4He elastic scattering, but overestimates the excitation energy of the 3+more » state by 350 keV. The bulk of the computed differential cross section is in good agreement with data. These results endorse the application of the present approach to the evaluation of the 2H(α,γ)6Li radiative capture, responsible for the big-bang nucleosynthesis of 6Li.« less

  15. Unified description of ^{6}Li structure and deuterium-^{4}He dynamics with chiral two- and three-nucleon forces.

    PubMed

    Hupin, Guillaume; Quaglioni, Sofia; Navrátil, Petr

    2015-05-29

    We provide a unified ab initio description of the ^{6}Li ground state and elastic scattering of deuterium (d) on ^{4}He (α) using two- and three-nucleon forces from chiral effective field theory. We analyze the influence of the three-nucleon force and reveal the role of continuum degrees of freedom in shaping the low-lying spectrum of ^{6}Li. The calculation reproduces the empirical binding energy of ^{6}Li, yielding an asymptotic D- to S-state ratio of the ^{6}Li wave function in the d+α configuration of -0.027, in agreement with a determination from ^{6}Li-^{4}He elastic scattering, but overestimates the excitation energy of the 3^{+} state by 350 keV. The bulk of the computed differential cross section is in good agreement with data. These results endorse the application of the present approach to the evaluation of the ^{2}H(α,γ)^{6}Li radiative capture, responsible for the big-bang nucleosynthesis of ^{6}Li.

  16. Frequency-dependent Study of Ultrapure Solid 4He by Using Rigid Double-pendulum Torsional Oscillator

    NASA Astrophysics Data System (ADS)

    Choi, Jaewon; Shin, Jaeho; Kim, Eunseong

    2015-03-01

    The physical origin of the period drop found in the torsional oscillator (TO) containing solid 4He was previously interpreted as the appearance of supersolidity. The current consensus is that the increase in the shear modulus leads to the period anomaly. Further studies show that the stiffening effect in TO can be amplified if a TO is not properly designed to be ``rigid.'' In this study, we designed a rigid double-pendulum TO. High purity solid 4He sample (0.6ppb) was grown by the block capillary method. The resonant period of TO starts to decrease from the empty cell data at 80mK. The ratio of the resonant period changes to the total mass loading are 3 . 8 ×10-5 and 2 . 6 ×10-4 for 1st and 2nd mode, respectively. Unlike recent experiment, we could not found a frequency-independent period drop. The upper bound for the putative supersolid fraction is less than 4 ×10-6 . The dissipation peak accompanied with the period drop was also analyzed with Cole-Cole plot and ωτ plot. We conclude that major contribution for the anomalous TO responses comes from the elastic effect.

  17. Unified description of ^{6}Li structure and deuterium-^{4}He dynamics with chiral two- and three-nucleon forces.

    PubMed

    Hupin, Guillaume; Quaglioni, Sofia; Navrátil, Petr

    2015-05-29

    We provide a unified ab initio description of the ^{6}Li ground state and elastic scattering of deuterium (d) on ^{4}He (α) using two- and three-nucleon forces from chiral effective field theory. We analyze the influence of the three-nucleon force and reveal the role of continuum degrees of freedom in shaping the low-lying spectrum of ^{6}Li. The calculation reproduces the empirical binding energy of ^{6}Li, yielding an asymptotic D- to S-state ratio of the ^{6}Li wave function in the d+α configuration of -0.027, in agreement with a determination from ^{6}Li-^{4}He elastic scattering, but overestimates the excitation energy of the 3^{+} state by 350 keV. The bulk of the computed differential cross section is in good agreement with data. These results endorse the application of the present approach to the evaluation of the ^{2}H(α,γ)^{6}Li radiative capture, responsible for the big-bang nucleosynthesis of ^{6}Li. PMID:26066431

  18. Studies of kinetic processes in a concentrated 3He-4He solution using an oscillating tuning fork

    NASA Astrophysics Data System (ADS)

    Bakhvalova, V. A.; Gritsenko, I. A.; Rudavskii, E. Ya.; Chagovets, V. K.; Sheshin, G. A.

    2015-07-01

    The dissipative processes causing the damping of quartz tuning fork vibrations in a solution of 15% 3He in 4He, are studied in a temperature range of 0.5-2.3 K. The resonance curves of the tuning forks are measured in the laminar flow region of the liquid, and their width is determined by the width of the dissipative processes. We examined tuning forks with a resonance frequency of 32 kHz, located inside a flask ("enclosed") and tuning forks without a flask ("unenclosed"). The results of the experiment are compared to existing theories. It was found that a significant contribution to the damping of tuning fork oscillations for a solution, as opposed to pure 4He, is from the second sound radiation, the contribution of which exceeds the input of viscous dissipation at low temperatures. The radiation of the first sound does not contribute to the damping of the oscillations of the "enclosed" fork due to the small size of the cell versus the wavelength. In the case of the "unenclosed" fork, the damping is determined by three processes: viscous dissipation and radiation of the first and second sounds.

  19. Airy minimum crossing θcm = 90° at Elab = 124 MeV for the 16O + 16O system

    NASA Astrophysics Data System (ADS)

    Kondo, Y.; Sugiyama, Y.; Tomita, T.; Yamanouchi, Y.; Ikezoe, H.; Ideno, K.; Hamada, S.; Sugimitsu, T.; Hijiya, M.; Fujita, H.

    1996-02-01

    We have measured the elastic scattering angular distribution for the 16O + 16O system at Elab = 124 MeV, where a prominent minimum has been observed in the θcm = 90° excitation function. The measured angular distribution shows modulated Airy structures at large angles with a dip at θcm = 90°. It is concluded that the prominent minimum in the excitation function is due to an Airy minimum, most likely to be the third member, crossing 90° at that energy.

  20. Low-3He/4He sublithospheric mantle source for the most magnesian magmas of the Karoo large igneous province

    NASA Astrophysics Data System (ADS)

    Heinonen, Jussi S.; Kurz, Mark D.

    2015-09-01

    The massive outpourings of Karoo and Ferrar continental flood basalts (CFBs) ∼180 Ma ago mark the initial Jurassic rifting stages of the Gondwana supercontinent. The origin and sources of these eruptions have been debated for decades, largely due to difficulties in defining their parental melt and mantle source characteristics. Recent findings of Fe- and Mg-rich dikes (depleted ferropicrite suite) from Vestfjella, western Dronning Maud Land, Antarctica, have shed light on the composition of the deep sub-Gondwanan mantle: these magmas have been connected to upper mantle sources presently sampled by the Southwest Indian Ocean mid-ocean ridge basalts (SWIR MORBs) or to high 3He/4He plume-entrained non-chondritic primitive mantle sources formed early in Earth's history. In an attempt to determine their He isotopic composition and relative contributions from magmatic, cosmogenic, and radiogenic He sources, we performed in-vacuo stepwise crushing and melting analyses of olivine mineral separates, some of which were abraded to remove the outer layer of the grains. The best estimate for the mantle isotopic composition is given by a sample with the highest amount of He released (>50%) during the first crushing step of an abraded coarse fraction. It has a 3He/4He of 7.03 ± 0.23 (2σ) times the atmospheric ratio (Ra), which is indistinguishable from those measured from SWIR MORBs (6.3-7.3 Ra; source 3He/4He ∼6.4-7.6 Ra at 180 Ma) and notably lower than in the most primitive lavas from the North Atlantic Igneous Province (up to 50 Ra), considered to represent the epitome magmas from non-chondritic primitive mantle sources. Previously published trace element and isotopic (Sr, Nd, and Pb) compositions do not suggest a direct genetic link to any modern hotspot of Indian or southern Atlantic Oceans. Although influence of a mantle plume cannot be ruled out, the high magma temperatures and SWIR MORB-like geochemistry of the suite are best explained by supercontinent insulation

  1. Parity-Violating Electron Scattering from {sup 4}He and the Strange Electric Form Factor of the Nucleon

    SciTech Connect

    Aniol, Konrad; Armstrong, David; Averett, Todd; Benaoum, Hachemi; Bertin, Pierre; Burtin, Etienne; Cahoon, Jason; Cates, Gordon; Chang, C; Chao, Yu-Chiu; Chen, Jian-Ping; Choi, Seonho; Chudakov, Eugene; Craver, Brandon; Cusanno, Francesco; Decowski, Piotr; Deepa, Deepa; Ferdi, Catherine; Feuerbach, Robert; Finn, John; Frullani, Salvatore; Fuoti, Kirsten; Garibaldi, Franco; Gilman, Ronald; Glamazdin, Oleksandr; Gorbenko, V; Grames, Joseph; Hansknecht, John; Higinbotham, Douglas; Holmes, Richard; Holmstrom, Timothy; Humensky, Thomas; Ibrahim, Hassan; Jager, Cornelis De; Jiang, Xiaodong; Kaufman, Lisa; Kelleher, Aidan; Kolarkar, Ameya; Kowalski, Stanley; Kumar, Krishna; Lambert, Daniel; Laviolette, Peter; LeRose, John; Lhuillier, David; Liyanage, Nilanga; Margaziotis, Demetrius; Mazouz, Malek; McCormick, Kathy; Meekins, David; Meziani, Zein-Eddine; Michaels, Robert; Moffit, Bryan; Monaghan, Peter; Camacho, Carlos Munoz; Nanda, Sirish; Nelyubin, Vladimir; Neyret, Damien; Paschke, Kent; Poelker, Benard; Pomatsalyuk, Roman; Qiang, Yi; Reitz, Bodo; Roche, Julie; Saha, Arunava; Singh, Jaideep; Snyder, Ryan; Souder, Paul; Subedi, Ramesh; Suleiman, Riad; Sulkosky, Vincent; Tobias, William; Urciuoli, Guido; Vacheret, Antonin; Voutier, Eric; Wang, Kebin; Wilson, R; Wojtsekhowski, Bogdan; Zheng, Xiaochao

    2005-06-01

    We have measured the parity-violating electroweak asymmetry in the elastic scattering of polarized electrons from {sup 4}He at an average scattering angle {theta}{sub lab} = 5.7 degrees and a four-momentum transfer Q{sup 2} = 0.091 GeV{sup 2}. From these data, for the first time, the strange electric form factor of the nucleon G{sub E}{sup s} can be isolated. The measured asymmetry of A{sub PV} = 6.72 {+-} 0.84 (stat) {+-} 0.21 (syst) parts per million yields a value of G{sub E}{sup s} = -0.038 {+-} 0.042 (stat) {+-} 0.010 (syst), consistent with zero.

  2. Capacitance-voltage studies of InP metal-oxide-semiconductor devices irradiated with 4He + ions

    NASA Astrophysics Data System (ADS)

    Tin, C. C.; Barnes, P. A.; Williams, J. R.; Patuwathavithane, C. S.; Van Staagen, P. K.

    1989-11-01

    Capacitance-voltage (C-V) measurements have been made on n-InP metal-oxide-semiconductor (MOS) devices damaged by 2-MeV 4 He+ ion bombardment. The C-V curves for samples with thin oxide layer (˜100 Å) show the presence of a depletion layer during both forward and reverse bias. This behavior is significantly different from those of normal, undamaged MOS devices. Measurements made on n-InP MOS samples with different oxide thicknesses show that the C-V curves gradually approach that of a MOS device on a p-type substrate. The anomalous behavior of the C-V curves for the irradiated samples can be explained by the presence of an n-p-n structure under the oxide layer.

  3. Acceptance Studies for 4He(e,e'p)X Reaction up to High Missing Energies and Momenta

    NASA Astrophysics Data System (ADS)

    Finton, Drew; Benmokhtar, Fatiha

    2014-03-01

    Data collected from the Helium-4 target in Hall A at Thomas Jefferson National Accelerator Facility (TJNAF) in Newport News, Virginia, was analyzed using the object-oriented data analysis software ROOT and used to create Missing Energy Spectra for Missing Momenta ranging from 150 MeV/c to 755 MeV/c for 4He(e,e'p)X reaction channels. Jefferson Lab is a continuous electron beam accelerator facility, and Hall A contains two high resolution spectrometers as well as the cryogenic Helium-4 target. Acceptance cuts were made to six measured variables to remove background noise, and then applied to produce a Missing Energy Spectrum showing two- and three-body break up channels as well as pion electro-production energy threshold. The analysis of these missing energy spectra will be used to understand the contributions of one-, two-, and three-body interactions.

  4. A Survey of Beam Asymmetries in Semi-exclusive Electron Scattering on {sup 4}He and {sup 12}C

    SciTech Connect

    Dan Protopopescu

    2002-12-01

    A study of the polarized electron beam asymmetry in semi-exclusive (e,e{prime}p) reactions on {sup 4}He and {sup 12}C over a large kinematic range has been performed. The beam asymmetry A{prime}{sub LT} is related to the imaginary part of the longitudinal-transverse interference and therefore it vanishes in reactions proceeding through a channel with a single dominant mechanism. In quasifree nucleon knockout, the helicity asymmetry provides an unambiguous signature for the interference between direct knockout and rescattering amplitudes. The data were taken in April-May 1999 using polarized beams of energies between 2.2 and 4.4 GeV, with the CEBAF Large Acceptance Spectrometer (CLAS) detector located in Hall B at the Jefferson Laboratory, VA. The measured asymmetries compare well with the theoretical predictions.

  5. Electric breakdown and ionization detection in normal liquid and superfluid 4He for the SNA nEDM experiment

    NASA Astrophysics Data System (ADS)

    Karcz, Maciej

    A new experiment to search for the neutron electric dipole moment (nEDM) is under construction at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory. The SNS nEDM experiment is a national collaboration spanning over 20 universities and laboratories with more than 100 physicists and engineers contributing to the research and development. The search for a nEDM is a precision test of time reversal symmetry in particle physics, in the absence of a discovery, the SNS nEDM experiment seeks to improve the present limit on the nEDM value by two orders of magnitude. A non-zero value of the nEDM would help to explain the asym- metry between matter and anti-matter in the universe by providing an additional source of charge conjugation and parity symmetry violation, a necessary ingredient in the theory of baryogenesis in the early universe. The nEDM experiment will measure the Larmor precession frequency of neutrons by detecting scintillation from neutron capture by a dilute concentration of 3He inside a bath of superfluid 4He. Neutron capture by 3He is spin-dependent and the magnetic moments of the neutron and the 3He nucleus are comparable. A direct measurement of the precession frequency of polarized 3He and scintillation from neutron capture allows for the relative precession frequencies of 3He and the neutron to be determined. The experiment will then look for changes in the relative precession of 3He and neutrons under the influence of strong electric fields. 3He has negligible EDM and therefore any deviation due to an applied electric field would be from a nEDM. The nEDM experiment will need to apply strong electric fields inside superfluid (SF) 4He and it was necessary to investigate the ability of SF 4He to sustain electric fields. An experiment to study electric breakdown in superfluid 4He was constructed at the Indiana University Center for Exploration of Energy and Matter (CEEM). The experiment studied the electric breakdown behavior of liquid

  6. Frequency-dependent study of solid 4He contained in a rigid double-torus torsional oscillator

    NASA Astrophysics Data System (ADS)

    Choi, Jaewon; Shin, Jaeho; Kim, Eunseong

    2015-10-01

    The rigid double-torus torsional oscillator (TO) is constructed to reduce any elastic effects inherent to complicated TO structures, allowing explicit probing for a genuine supersolid signature. We investigated the frequency- and temperature-dependent response of the rigid double-torus TO containing solid 4He with 0.6-ppb 3He and 300-ppb 3He . We did not find evidence to support the frequency-independent contribution proposed to be a property of supersolid helium. The frequency-dependent contribution which comes from the simple elastic effect of solid helium coupled to the TO is essentially responsible for the entire response. The magnitude of the period drop is linearly proportional to f2, indicating that the responses observed in this TO are mostly caused by the overshoot of "soft" solid helium against the wall of the torus. Dissipation of the rigid TO is vastly suppressed compared to that of nonrigid TOs.

  7. Frequency stabilization of a 1083 nm fiber laser to {sup 4}He transition lines with optical heterodyne saturation spectroscopies

    SciTech Connect

    Gong, W.; Peng, X. Li, W.; Guo, H.

    2014-07-15

    Two kinds of optical heterodyne saturation spectroscopies, namely, frequency modulation spectroscopy (FMS) and modulation transfer spectroscopy (MTS), are demonstrated for locking a fiber laser to the transition lines of metastable {sup 4}He atoms around 1083 nm. The servo-loop error signals of FMS and MTS for stabilizing laser frequency are optimized by studying the dependence of the peak-to-peak amplitude and slope on the optical power of pump and probe beams. A comparison of the stabilization performances of FMS/MTS and polarization spectroscopy (PS) is presented, which shows that MTS exhibits relatively superior performance with the least laser frequency fluctuation due to its flat-background dispersive signal, originated from the four-wave mixing process. The Allan deviation of the stabilized laser frequency is 5.4 × 10{sup −12}@100 s with MTS for data acquired in 1000 s, which is sufficiently applicable for fields like laser cooling, optical pumping, and optical magnetometry.

  8. Frequency stabilization of a 1083 nm fiber laser to 4He transition lines with optical heterodyne saturation spectroscopies

    NASA Astrophysics Data System (ADS)

    Gong, W.; Peng, X.; Li, W.; Guo, H.

    2014-07-01

    Two kinds of optical heterodyne saturation spectroscopies, namely, frequency modulation spectroscopy (FMS) and modulation transfer spectroscopy (MTS), are demonstrated for locking a fiber laser to the transition lines of metastable 4He atoms around 1083 nm. The servo-loop error signals of FMS and MTS for stabilizing laser frequency are optimized by studying the dependence of the peak-to-peak amplitude and slope on the optical power of pump and probe beams. A comparison of the stabilization performances of FMS/MTS and polarization spectroscopy (PS) is presented, which shows that MTS exhibits relatively superior performance with the least laser frequency fluctuation due to its flat-background dispersive signal, originated from the four-wave mixing process. The Allan deviation of the stabilized laser frequency is 5.4 × 10-12@100 s with MTS for data acquired in 1000 s, which is sufficiently applicable for fields like laser cooling, optical pumping, and optical magnetometry.

  9. Ratios of 15N/12C and 4He/12C inclusive electroproduction cross sections in the nucleon resonance region

    SciTech Connect

    Peter Bosted; Robert Fersch

    2007-12-14

    The ratio of inclusive electron scattering cross sections for 15N/12C was determined in the kinematic range 0.8<2 GeV and 0.2<1 GeV2 using 2.285 GeV electrons and the CLAS detector at Jefferson Lab. The ratio exhibits only slight resonance structure, as predicted by a phenomenological model, and also by quark-hadron duality. Within the super-scaling quasi-elastic model, slight evidence is found for a 1 MeV lower effective nucleon binding energy in 15N than in 12C. Ratios of 4He/12C using 1.6 to 2.5 GeV electrons are in good agreement with the phenomenological model.

  10. Parity-Violating Electron Scattering from {sup 4}He and the Strange Electric Form Factor of the Nucleon

    SciTech Connect

    Aniol, K.A.; Margaziotis, D.J.; Armstrong, D.S.; Averett, T.; Finn, J.M.; Holmstrom, T.; Kelleher, A.; Moffit, B.; Sulkosky, V.; Benaoum, H.; Holmes, R.; Souder, P.A.; Bertin, P.Y.; Ferdi, C.

    2006-01-20

    We have measured the parity-violating electroweak asymmetry in the elastic scattering of polarized electrons from {sup 4}He at an average scattering angle <{theta}{sub lab}>=5.7 deg. and a four-momentum transfer Q{sup 2}=0.091 GeV{sup 2}. From these data, for the first time, the strange electric form factor of the nucleon G{sub E}{sup s} can be isolated. The measured asymmetry of A{sub PV}=(6.72{+-}0.84{sub (stat)}{+-}0.21{sub (syst)})x10{sup -6} yields a value of G{sub E}{sup s}=-0.038{+-}0.042{sub (stat)}{+-}0.010{sub (syst)}, consistent with zero.

  11. Nonlinear Transport of the Wigner Crystal on Superfluid 4He in a Quasi-One-Dimensional Channel

    NASA Astrophysics Data System (ADS)

    Vasylenko, Anna A.; Misko, Vyacheslav R.

    2014-07-01

    We study transport properties of a Wigner crystal driven by an external force on the surface of superfluid 4He, in the "quantum wire" regime, i.e. in the quasi-one-dimensional (quasi-1D) case when a typical width of the channel is comparable to the inter-electron separation. Utilizing molecular dynamics simulations, we investigate the electronic transport through the channels with different constrictions: (i) geometrical constrictions with varying shape and size, and (ii) a saddle-point potential with varying gate voltage. The average particle velocity has been calculated as a function of the driving force or gate voltage. We have revealed a significant difference in the dynamical behavior for long and short constrictions. In particular, we found that the oscillations of the average particle velocity in channels with short constrictions exhibit a clear correlation with the transitions between the states with different numbers of rows of particles in the constriction, while for channels with longer constrictions these oscillations are suppressed. The obtained results are in agreement with the recent experimental observations,1 and thus bring new important insights into the dynamics of electrons floating on the surface of superfluid 4He in channels with constrictions. Special Issue Comments: This article presents results on the dynamics of electrons moving on the surface of liquid helium in narrow channels with constrictions, with a focus on the "quantum wire", i.e. single file, regime. This article is connected to the Special Issue articles about advanced statistical properties in single file dynamics39 and the experiments on liquid helium.40

  12. Correlation of gold in siliceous sinters with 3He 4He in hot spring waters of Yellowstone National Park

    USGS Publications Warehouse

    Fournier, R.O.; Kennedy, B.M.; Aoki, M.; Thompson, J.M.

    1994-01-01

    temperatures may contain waters with different [H2S] and [Au]. The [H2S] in a subsurface reservoir water is difficult to assess on the basis of analyses of hot spring waters because of uncertainties about steam loss during fluid ascent. However, the same processes that result in low [H2S] in reservoir waters also tend to result in decreases in the ratio of 3He 4He(R) dissolved in that water. Values of R relative to this ratio in air (Ra) attain values > 15 in YNP thermal waters. To date, all of the thermal waters at YNP that have R Ra values <9 have been found to deposit sinters with relatively low gold concentrations. These include all of the thermal waters that discharge from 180-215??C reservoirs at Upper, Midway, and Lower Geyser Basins within the western part of the Yellowstone caldera, and thermal waters at Norris Geyser Basin, outside the Yellowstone caldera, where some of the waters flow directly to the surface from a reservoir where the temperature is about 300??C. A high 3He 4He ratio in thermal water discharged at the surface does not guarantee high gold concentrations in the sinter deposited by this water. Boiling with loss of steam (the gas phase takes a separate route to the surface) during rapid upflow from the shallowest reservoir to the surface decreases the [H2S] and total He dissolved in the residual liquid without appreciably changing the 3He 4He ratio. This is because the isotopic composition of the He of the initial bulk fluid is unchanged and there is too little time for much radiogenic 4He to build back into the liquid during this rapid ascent from the near-surface reservoir. However, if boiling with phase separation and loss of steam occurs deep in the system, the 3He 4He ratio in the residual liquid, now depleted in H2S and total He, will be susceptible to dilution with radiogenic 4He that is acquired during the longer residence time underground. Some or all of the Au that comes out of solution when an initial gold bisulfide complex breaks

  13. Comparison of the effectiveness of exposure to low LET helium particles (4He) and gamma rays (137Cs) on the disruption of cognitive performance

    Technology Transfer Automated Retrieval System (TEKTRAN)

    Rats were exposed to either Helium (4He) particles (1000 MeV/n; 0.1 – 10 cGy; head-only) or Cesium 137Cs gamma rays (50 – 400 cGy; whole body) and the effects of irradiation on cognitive performance evaluated. The results indicated that exposure to doses of 4He particles as low as 0.1 cGy disrupted...

  14. Uptake of [3H]-nicotine and [3H]-noradrenaline by cultured chromaffin cells.

    PubMed Central

    Ceña, V.; García, A. G.; Montiel, C.; Sánchez-García, P.

    1984-01-01

    Three day-old cultured bovine adrenal chromaffin cells incubated at room temperature with Krebs-HEPES solution containing different concentrations of [3H]-nicotine, took up and retained increasing amounts of the drug by a mechanism that did not saturate. Concentrations of cold nicotine as high as 100 microM did not alter the amount of [3H]-nicotine retained by cells. Imipramine, cocaine, tetracaine or mecamylamine, at concentrations (10 microM) that blocked the catecholamine secretory effects of nicotine completely, did not modify the uptake of [3H]-nicotine. Both imipramine and cocaine drastically inhibited [3H]-noradrenaline uptake by cells in a concentration-dependent manner (IC50S of 0.08 and 1 microM, respectively). These data indicate that the secretory effects of nicotine are not coupled to its previous uptake into cells, and are evidence in favour of a site of action for nicotine located in or at the surface of the chromaffin cell membrane. PMID:6704577

  15. Construction of a Newly Designed Small-Size Mass Spectrometer for Helium Isotope Analysis: Toward the Continuous Monitoring of 3He/4He Ratios in Natural Fluids

    PubMed Central

    Bajo, Ken-ichi; Sumino, Hirochika; Toyoda, Michisato; Okazaki, Ryuji; Osawa, Takahito; Ishihara, Morio; Katakuse, Itsuo; Notsu, Kenji; Igarashi, George; Nagao, Keisuke

    2012-01-01

    The construction of a small-size, magnetic sector, single focusing mass spectrometer (He-MS) for the continuous, on-site monitoring of He isotope ratios (3He/4He) is described. The instrument is capable of measuring 4He/20Ne ratios dissolved in several different types of natural fluids of geochemical interest, such as groundwater and gas from hot springs, volcanoes and gas well fields. The ion optics of He-MS was designed using an ion trajectory simulation program “TRIO,” which permits the simultaneous measurement of 3He and 4He with a double collector system under a mass resolution power (M/ΔM) of >700. The presently attained specifications of He-MS are; (1) a mass resolving power of ca. 430, sufficient to separate 3He+ from interfering ions, HD+ and H3+, (2) ultra-high vacuum conditions down to 3×10−8 Pa, and (3) a sufficiently high sensitivity to permit amounts of 3He to be detected at levels as small as 10−13 cm3 STP (3×106 atoms). Long term stability for 3He/4He analysis was examined by measuring the 3He/4He standard gas (HESJ) and atmospheric He, resulting in ∼3% reproducibility and ≤5% experimental error for various amounts of atmospheric He from 0.3 to 2.3×10−6 cm3 STP introduced into the instrument. A dynamic range of measurable 3He/4He ratios with He-MS is greater than 103 which was determined by measuring various types of natural fluid samples from continental gas (with a low 3He/4He ratio down to 2×10−8) to volcanic gas (with a high 3He/4He ratio up to 3×10−5). The accuracy and precision of 3He/4He and 4He/20Ne ratios were evaluated by comparing the values with those measured using well established noble gas mass spectrometers (modified VG5400/MS-III and -IV) in our laboratory, and were found to be in good agreement within analytical errors. Usefulness of the selective extraction of He from water/gas using a high permeability of He through a silica glass wall at high temperature (700°C) is demonstrated. PMID:24349910

  16. Characterization of helium diffusion behavior from continuous heating experiments: Sample screening and identification of multiple 4He components

    NASA Astrophysics Data System (ADS)

    McDannell, K. T.; Idleman, B. D.; Zeitler, P. K.

    2015-12-01

    Old, slowly cooled apatites often yield overdispersed helium ages due to factors such as parent zonation, He implantation, radiation damage, crystal defects, and fluid inclusions. Careful mineral selection and many replicate analyses can mitigate the impact of some of these effects. However, this approach adds unnecessary costs in time and resources when dating well-behaved apatites and is generally ineffective at identifying the root cause of age dispersion and providing suitable age corrections for poorly behaved samples. We assess a new technique utilizing static-gas measurement during continuous heating as a means to rapidly screen apatite samples. In about the time required for a conventional total-gas analysis, this method can discriminate between samples showing the volume-diffusion behavior expected for apatite and those showing anomalous release patterns, inconsistent with their use in thermochronologic applications. This method may also have the potential to quantify and discriminate between the radiogenic and extraneous 4He fractions released by a sample. Continuously heated samples that outgas by volume diffusion during a linear heating schedule should produce a characteristic sigmoidal 4He fractional loss profile, with the exact shape and position of these profiles (in loss vs. heating time space) controlled by sample kinetics, grain size, and heating rate. Secondary factors such as sample zoning and alpha-loss distribution have a relatively minor impact on such profiles. Well-behaved examples such as the Durango standard and other apatites with good age reproducibility show the expected smooth, sigmoidal gas release with complete exhaustion by temperatures predicted for volume diffusion using typical apatite kinetics (e.g., by ~900˚C for linear heating at 20˚C/minute). In contrast, "bad actor" samples that do not replicate well show significant degrees of helium release deferred to higher temperatures. We report on screening results for a range of

  17. 3H-nicotine, 3H-flunitrazepam, and 3H-cocaine incorporation into melanin: a model for the examination of drug-melanin interactions.

    PubMed

    Claffey, D J; Stout, P R; Ruth, J A

    2001-10-01

    To explore drug-melanin interactions, we examined the in vitro tyrosinase-mediated formation of melanin from tyrosine in the presence of the 3H-cocaine (3H-COC), 3H-flunitrazepam (3H-FLU), and 3H-nicotine (3H-NIC) at 10-100,000 ng/mL. Polymerization in the presence of 10 or 100 ng/mL of each drug resulted in almost complete drug incorporation into the melanin pellet. Only 12% (3H-NIC) to 28% (3H-FLU) of the pellet-associated radioactivity could be released upon treatment with 6 M HCl. At 1000-100,000 ng/mL, between 20 and 50% of label became melanin-associated. In each case a significant percentage of melanin-associated radioactivity was resistant to treatment with 6 M HCl. Nicotine-associated radioactivity in the polymer was subject to much greater quenching than was 3H-COC or 3H-FLU, suggesting a much tighter association with the melanin. The subsequent demonstration of a covalent adduct of a melanin intermediate and nicotine has demonstrated the utility of this polymerization system as a model for further chemical characterization of drug-melanin interactions.

  18. On the K- 4He → Λπ- 3He resonant and non-resonant processes

    NASA Astrophysics Data System (ADS)

    Piscicchia, K.; Wycech, S.; Curceanu, C.

    2016-10-01

    The ongoing data analyses by the AMADEUS/KLOE-2 Collaboration on the 2004-2005 KLOE data revive studies of the K ‾ nuclear absorption at low energies. The aim is to study K ‾ interactions at subthreshold energies and to search for signals of K ‾ meson nuclear states. In this paper the spectrum of the K- 4He → Λπ- 3He reaction is discussed. One - calculable - mode of decay involves P-wave intermediate Σ (1385) resonance. Another mode involves S-wave KN → Λπ amplitude which may be extracted from the experimental results. Comparison of these two allows a check of subthreshold extrapolations of multichannel K ‾ N S-wave interaction models. Given the established significance of the P wave interaction in the K ‾ N system presented here, the obtained spectra will serve for the AMADEUS/KLOE-2 data analysis, in order to properly extract the subthreshold non-resonant transition amplitude.

  19. Mutual interactions between objects oscillating in isotopically pure superfluid 4He in the T → 0 limit

    NASA Astrophysics Data System (ADS)

    Garg, D.; Efimov, V. B.; Giltrow, M.; McClintock, P. V. E.; Skrbek, L.

    2012-11-01

    We report the results of experiments to explore interactions between physically separated oscillating objects in isotopically pure superfluid 4He at T ˜ 10 mK. The investigations focused mainly on 32 kHz quartz tuning forks, but also consider a nearby 1 kHz oscillating grid. The low-drive linewidth (LDL) and resonant frequency fd of a detector fork were monitored while the maximum velocity of a transmitter fork, separated from the detector by a few mm, was varied over a wide range. Clear evidence was found for mutual interactions between the two forks, and for the influence of the grid on the forks. Monitoring the detector's LDL and fd provides evidence for a generator critical velocity in the range 0.3<υc1<1.0 cm/s for onset of the detector responses, in addition to a second critical velocity υc2˜13 cm/s probably corresponding to the production of quantum turbulence at the generator. The results are discussed, but are not yet fully understood.

  20. A "high 4He/3He" mantle material detected under the East Pacific Rise (15°4'N)

    NASA Astrophysics Data System (ADS)

    Mougel, Berengere; Moreira, Manuel; Agranier, Arnaud

    2015-03-01

    We investigate in details helium isotope data reported in Mougel et al. (2014) for 14 basaltic samples collected on the East Pacific Rise by submersible (15°4'N) where the ridge interacts with the Mathematician seamounts. Samples locations are separated by only few hundred meters across a 15 km along-axis profile. The data reveal a strong geochemical variability that has never been observed at such high spatial resolution for helium isotope compositions. Moreover, they reveal an unusually high 4He/3He mantle component also characterized by unradiogenic lead, atypical in oceanic basalts. He-Pb systematics suggests a mixture between a nonradiogenic lead and radiogenic helium pyroxenitic component, recycled from the deep continental lithosphere and the ambient peridotitic mantle. The He isotope difference between these two end-members can be interpreted as a time evolution of two distinct mantle sources after a slight (U + Th)/3He fractionation, likely due to some ancient degassing during the formation of deep continental pyroxenites.

  1. Experimental realization of the zero temperature Random Field Ising Model : the condensation of 4He in aerogels

    NASA Astrophysics Data System (ADS)

    Aubry, Geoffroy; Guyon, Laurent; Melich, Mathieu; Spathis, Panayotis; Despetis, Florence; Wolf, Pierre-Etienne

    2013-03-01

    Although widely studied, the effect of disorder on a first order phase transition is still highly debated. Numerical simulations of the T = 0 Random Field Ising Model show that magnetization evolves by avalanches, the average size of which diverges below a critical disorder (Sethna et al., PRL 70 3347 (1993)). Nevertheless, experimental evidence is scarce up to now (Berger et al., PRL 85, 4176 (2000)). In the case of the liquid gas transition in disordered porous media, the same theoretical concepts can be applied (Detcheverry et al., PRE 72 051506 (2005)). We have studied experimentally this phase transition using 4He in silica aerogels. Optical and thermodynamical measurements show that the condensation is an out of equilibrium process. We clearly observe two filling regimes separated by a critical temperature T* : below T*, filling is discontinuous (macro avalanche) whereas above T* it becomes continuous (micro avalanches). In addition, we have developed a speckle interferometry technique to detect single avalanches. We argue that our results support the disorder induced phase transition. This work was supported by ANR-06-BLAN-0098.

  2. Development of GM cryocooler separate type liquid-helium-free 3He-4He dilution refrigerator system

    NASA Astrophysics Data System (ADS)

    Yamanaka, Y.; Ito, T.; Umeno, T.; Suzuki, Y.; Yoshida, S.; Kamioka, Y.; Maehata, K.

    2009-02-01

    We developed the new liquid-helium-free dilution refrigerator system, in which the Gifford-McMahon (GM) cycle cryocooler and dilution refrigerator (DR) unit are separated. We obtained the base temperature below 50 mK in this DR system. In usual liquid-helium-free DR systems, the DR unit directly couples with GM-cryocooler in the same vacuum chamber. Therefore the mechanical vibration of GM-cryocooler is hardly removed from DR unit. In order to eliminate the vibration problem, the separated vacuum chamber contacting the GM-cryocooler is connected with the DR unit chamber by the flexible hose with length of about 1 meter. Thin flexible tubes used for circulation of the refrigerant gas and radiation shield are installed in the connection hose. The 4He gas, cooled in the GM-cryocooler unit, transfers to the DR unit throw the thin flexible tubes. After cooling the DR unit, the gas returns to GM-cryocooler unit with cooling of the radiation shield. We expect that our separate-type dilution refrigerator becomes a useful piece of apparatus for the low temperature experiments.

  3. Study of astrophysically important resonant states in 26Si by the 28Si(4He,6He)26Si reaction

    NASA Astrophysics Data System (ADS)

    Kwon, Young Kwan; Lee, C. S.; Moon, J. Y.; Lee, J. H.; Kim, J. Y.; Kubono, S.; Iwasa, N.; Inafiki, K.; Yamaguchi, H.; He, J. J.; Saito, A.; Wakabayashi, Y.; Fukijawa, H.; Amadio, G.; Khiem, L. H.; Tanaka, M.; Chen, A.; Kato, S.

    PoS(NIC-IX)024 , b, H. Yamaguchia, J. J. Hea , A. Saitoa , Y. Wakabayashia, H. Fujikawaa, G. The emission of 1.809 MeV gamma-ray from the first excited state of 26 Mg followed by beta- decay of 26 Al in its ground state (denoted as 26 Alg.s. ) has been identified by gamma-ray telescopes such the Compton Gamma-Ray Observatory (CGRO) [1]. To resolve controversy over the pos- sible sources of the observational 1.809 MeV gamma-rays, one needs accurate knowledge of the production rate of 26 Al. The 25 Al(p,γ)26Si reaction which is the competition reaction for produc- tion of 26 Alg.s. is one of the important subjects to be investigated. In this work, the astrophysically important 26 Si states above the proton threshold were studied via the 28 Si(4 He,6 He)26 Si reaction. We have preformed an angular distribution measurement using the high resolution QDD spectro- graph (PA) at Center for Nuclear Study (CNS), University of Tokyo. The experimental results and data analysis will be presented.

  4. Differential binding of /sup 3/H-imipramine and /sup 3/H-mianserin in rat cerebral cortex

    SciTech Connect

    Dumbrille-Ross, A.; Tang, S.W.; Coscina, D.V.

    1981-11-16

    Drug competition profiles, effect of raphe lesion, and sodium dependency of the binding of two antidepressant drugs /sup 3/H-imipramine and /sup 3/H-mianserin to rat cerebral cortex homogenate were compared to examine whether the drugs bound to a common ''antidepressant receptor.'' Of the neurotransmitters tested, only serotonin displaced binding of both /sup 3/H-imipramine and /sup 3/H-mianserin. /sup 3/H-Mianserin binding was potently displaced by serotonin S/sub 2/ antagonists and exhibited a profile similar to that of /sup 3/H-spiperone binding. In the presence of the serotonin S/sub 2/ antagonist spiperone, antihistamines (H/sub 1/) potently displaced /sup 3/H-mianserin binding. /sup 3/H-Imipramine binding was displaced potently by serotonin uptake inhibitors. The order of potency of serotonergic drugs in displacing /sup 3/H-imipramine binding was not similar to their order in displacing /sup 3/H-spiperone or -3H-serotonin binding. Prior midbrain raphe lesions greatly decreased the binding of /sup 3/H-imipramine but did not alter binding of /sup 3/H-mianserin. Binding of /sup 3/H-imipramine but not /sup 3/H-mianserin was sodium dependent. These results show that /sup 3/H-imipramine and /sup 3/H-mianserin bind to different receptors. /sup 3/H-Imipramine binds to a presynaptic serotonin receptor which is probably related to a serotonin uptake recognition site, the binding of which is sodium dependent. /sup 3/H-Mianserin binds to postsynaptic receptors, possibly both serotonin S/sub 2/ and histamine H/sub 1/ receptors, the binding of which is sodium independent.

  5. Indirect study of 12C(α,γ)16O reaction

    NASA Astrophysics Data System (ADS)

    Hammache, F.; Oulebsir, N.; Roussel, P.; Pellegriti, M. G.; Audouin, L.; Beaumel, D.; Bouda, A.; Descouvemont, P.; Fortier, S.; Gaudefroy, L.; Kiener, J.; Lefebvre-Schuhl, A.; Tatischeff, V.

    2016-01-01

    The radiative capture reaction 12C(α,γ)16O plays an important role in helium burning in massive stars and their subsequent evolution [1]. However, despite various experimental studies, the cross section of this reaction at stellar energies remains highly uncertain. The extrapolation down to stellar energy (Ecm˜300 keV) of the measured cross sections at higher energies is made difficult by the overlap of various contributions of which some are badly known such as that of the 2+ (Ex=6.92 MeV) and 1- (Ex=7.12 MeV) sub-threshold states of 16O. Hence, to further investigate the contribution of these two-subthreshold resonances to the 12C(α,γ)16O cross section, a new determination of their a-reduced widths and so their a- spectroscopic-factors was performed using 12C(7Li,t)16O transfer reaction measurements at two incident energies and a detailed DWBA analysis of the data [2]. The measured and calculated differential cross sections are presented as well as the obtained spectroscopic factors and the a- reduced widths as well as the assymptotic normalization constants (ANC) for the 2+ and 1- subthreshold states. Finally, the results obtained from the R-matrix calculations of the 12C(α,γ)16O cross section using our obtained a-reduced widths for the two sub-threshold resonances are presented and discussed.

  6. An Experimental Study on What Controls the Ratios of 18O/16O and 17O/16O of O2 During Microbial Respiration

    NASA Astrophysics Data System (ADS)

    Stolper, D. A.; Ward, B. B.; Fischer, W. W.; Bender, M. L.

    2015-12-01

    18O/16O and 17O/16O ratios of atmospheric and dissolved oceanic O2 are key biogeochemical tracers of total photosynthesis and respiration on global to local length scales and glacial/interglacial time scales (Luz et al., 1999). Critical to the use of these ratios as biogeochemical tracers is knowledge of how they are affected by production, consumption, and transport of O2. We present new measurements of O2 respiration by E. coli and N. oceanus, an ammonia oxidizing bacterium, to test three assumptions of isotopically enabled models of the O2 cycle: (i) laboratory-measured respiratory 18O/16O isotope effects (18α) of microorganisms are constant under all experimental and natural conditions (e.g., temperature and growth rate); (ii) the respiratory 'mass law' relationship between 18O/16O and 17O/16O [17α = (18α)β] is universal; and (iii) 18α and β for aerobic ammonia and organic carbon oxidation are identical. For E. coli, we find that both 18α and β are variable. From 37°C to 15°C, 18α varies linearly with temperature from 17 to 14‰, and β varies linearly from 0.513 to 0.508. 18α and β do not appear to vary with growth rate (as tested using different carbon sources). Both 18α and β are lower than previous observations for bacteria: 18α = 17-20‰ (Kiddon et al., 1993) and β = 0.515 (Luz and Barkan, 2005). We were able to simulate the observed temperature dependence of 18α and β using a model of respiration with two isotopically discriminating steps: O2 binding to cytochrome bo oxidase (the respiratory enzyme) and reduction of O2 to H2O. Finally, initial results on N. oceanus suggest it has similar values for 18α and β as previously studied aerobic bacteria that consume organic carbon, providing the first support for assumption (iii). Based on these results, isotopically constrained biogeochemical models of O2 cycling may need to consider a temperature dependence for 18α and β for microbial respiration. For example, these results may

  7. Bare-nucleus astrophysical factor of the {sup 3}He(d,p){sup 4}He reaction via the 'Trojan horse' method

    SciTech Connect

    La Cognata, M.; Spitaleri, C.; Tumino, A.; Cherubini, S.; Lamia, L.; Musumarra, A.; Pizzone, R.G.; Rinollo, A.; Romano, S.; Typel, S.; Rolfs, C.; Schuermann, D.; Strieder, F.

    2005-12-15

    The {sup 3}He(d,p){sup 4}He reaction has been studied from E{sub c.m.}=600 keV down to astrophysical energies by means of the 'Trojan horse' method using the {sup 6}Li({sup 3}He,p{alpha}){sup 4}He three-body reaction at E{sub lab}=5 and 6 MeV. Coincidence spectra were measured in kinematic conditions favoring the quasifree {sup 3}He+{sup 2}H process. The bare astrophysical factor S{sub b}(E) for the {sup 3}He(d,p){sup 4}He reaction was extracted from the three-body cross section in the modified plane-wave Born approximation. Comparison with the S{sub b} extrapolation from the free two-body data is presented. The independent estimate of the screening potential as obtained with the present work seems to confirm the theoretical adiabatic limit.

  8. Measurement of the {sup 12}C({alpha},{gamma}){sup 16}O reaction at TRIAC

    SciTech Connect

    Makii, H.; Miyatake, H.; Wakabayashi, Y.; Ishiyama, H.; Niki, K.; Okada, M.; Imai, N.; Watanabe, Y. X.; Hirayama, Y.; Jeong, S. C.; Shima, T.; Nishinaka, I.; Mitsuoka, S.; Nishio, K.; Chiba, S.

    2012-11-12

    We have measured the {gamma}-ray angular distribution of the {sup 12}C({alpha},{gamma}){sup 16}O reaction at TRIAC (Tokai Radioactive Ion Accelerator Complex) to accurately determine the E1 and E2 cross sections. In this experiment, we used high efficiency anti-Compton NaI(T1) spectrometers to detect a {gamma}-ray from the reaction with large S/N ratio, intense pulsed {alpha}-beams to discriminate true event from background events due to neutrons from {sup 13}C({alpha},n){sup 16}O reaction with a time-of-flight (TOF) method. We succeeded in removing a background events due to neutrons and clearly detected {gamma}-ray from the {sup 12}C({alpha}{gamma}){sup 16}O reaction with high statistics.

  9. Fragment angular correlation in the breakup of 16O ions at 95 MeV/A

    NASA Astrophysics Data System (ADS)

    Tatischeff, V.; Kiener, J.; Aguer, P.; Bogaert, G.; Coc, A.; Disdier, D.; Ichihara, T.; Kraus, L.; Lefebvre, A.; Linck, I.; Mittig, W.; Motobayashi, T.; de Oliveira Santos, F.; Roussel-Chomaz, P.; Stephan, C.; Thibaud, J. P.

    1998-04-01

    Fragment angular correlations in projectile breakup reactions are very sensitive to interference between different multipolarities entering in the excitation-dissociation process of the projectile. In particular, it was proposed to disentangle L=1 and L=2 contributions in direct breakup reactions of 16O with low relative energy between the α and 12C fragment, which are of astrophysical interest. We studied the experimental aspects of extracting those angular correlations in extreme kinematical conditions usually encountered in breakup experiments of astrophysical interest. The breakup of 95 MeV/A 16O projectiles induced by a 208Pb target was measured using the high-resolution spectrometer SPEG at Ganil for the coincident detection of the fragments. Sequential breakup via the 12.53 MeV level of 16O is analyzed in this framework and it favors an one-step M2 excitation of this level.

  10. Long-distance correlation-length effects and hydrodynamics of 4He films in a Corbino geometry

    NASA Astrophysics Data System (ADS)

    Thomson, Stephen R. D.; Perron, Justin K.; Gasparini, Francis M.

    2016-09-01

    Previous measurements of the superfluid density ρs and specific heat for 4He have identified effects that are manifest at distances much larger than the correlation length ξ3 D [Perron et al., Nat. Phys. 6, 499 (2010), 10.1038/nphys1671; Perron and Gasparini, Phys. Rev. Lett. 109, 035302 (2012), 10.1103/PhysRevLett.109.035302; Perron et al., Phys. Rev. B 87, 094507 (2013), 10.1103/PhysRevB.87.094507]. We report here measurements of the superfluid density which are designed to explore this phenomenon further. We determine the superfluid fraction ρs/ρ from the resonance of 34-nm films of varying widths 4 ≤W ≤100 μ m . The films are formed across a Corbino ring separating two chambers where a thicker 268-nm film is formed. This arrangement is realized using lithography and direct Si-wafer bonding. We identify two effects in the behavior of ρs/ρ : one is hydrodynamic, for which we present an analysis, and the other is a correlation-length effect which manifests as a shift in the transition temperature Tc relative to that of a uniform 34-nm film uninfluenced by proximity effects. We find that one can collapse both ρs/ρ and the quality factor of the resonance onto universal curves by shifting Tc as Δ Tc˜W-ν . This scaling is a surprising result on two counts: it involves a very large length scale W relative to the magnitude of ξ3 D and the dependence on W is not what is expected from correlation-length finite-size scaling which would predict Δ Tc˜W-1 /ν .

  11. Human epididymis protein 4 (HE4) plays a key role in ovarian cancer cell adhesion and motility

    SciTech Connect

    Lu, Renquan; Sun, Xinghui; Xiao, Ran; Zhou, Lei; Gao, Xiang; Guo, Lin

    2012-03-09

    Highlights: Black-Right-Pointing-Pointer We generated stable transduced HE4 overexpression and knockdown cells. Black-Right-Pointing-Pointer HE4 was associated with EOC cell adhesion and motility. Black-Right-Pointing-Pointer HE4 might have some effects on activation of EGFR-MAPK signaling pathway. Black-Right-Pointing-Pointer HE4 play an important role in EOC tumorigenicity. -- Abstract: Human epididymis protein 4 (HE4) is a novel and specific biomarker for epithelial ovarian cancer (EOC). We previously demonstrated that serum HE4 levels were significantly elevated in the majority of EOC patients but not in subjects with benign disease or healthy controls. However, the precise mechanism of HE4 protein function is unknown. In this study, we generated HE4-overexpressing SKOV3 cells and found that stably transduced cells promoted cell adhesion and migration. Knockdown of HE4 expression was achieved by stable transfection of SKOV3 cells with a construct encoding a short hairpin DNA directed against the HE4 gene. Correspondingly, the proliferation and spreading ability of HE4-expressed cells were inhibited by HE4 suppression. Mechanistically, impaired EGFR and Erk1/2 phosphorylation were observed in cells with HE4 knockdown. The phosphorylation was restored when the knockdown cells were cultured in conditioned medium containing HE4. Moreover, in vivo tumorigenicity showed that HE4 suppression markedly inhibited the growth of tumors. This suggests that expression of HE4 is associated with cancer cell adhesion, migration and tumor growth, which can be related to its effects on the EGFR-MAPK signaling pathway. Our results provide evidence of the cellular and molecular mechanisms that may underlie the motility-promoting role of HE4 in EOC progression. The role of HE4 as a target for gene-based therapy might be considered in future studies.

  12. Relation between (e, e') sum rules in 6, 7Li and 4He nuclei: Experiment and cluster model

    NASA Astrophysics Data System (ADS)

    Efros, V. D.; Timchenko, I. S.; Buki, A. Yu.

    2016-09-01

    The sums over ( e, e') spectra of 6Li and 7Li nuclei which correspond to the longitudinal sum rule are studied. It is suggested that due to the cluster structure of the lithium isotopes these sums may approximately be expressed in terms of such a sum pertaining to the α-particle. Calculation of these sums is performed in the framework of cluster models with antisymmetrization done with respect to all the nucleons. At momentum transfers higher than 0.8 fm-1 the relations expressing the A = 6 or 7 sum in terms of the A = 4 sum prove to be valid with rather high accuracy. In the region of momentum transfers around 1 fm-1 the longitudinal correlation functions of 6Li and 7Li nuclei are found to be close to that of the α-particle. Basing on this, the difference between the q values at which the high- q limit of the inelastic sum rule is reached in the 6, 7Li cases and the 4He case is explained. The experimental longitudinal sums in the range between 0.450 and 1.625 fm-1 are employed to perform comparison with the theoretical sum rule calculated in the framework of cluster models. Out of the experimental sums, those in the range between 0.750 and 1.000 fm-1 in the 6Li case and between 0.750 and 1.125 fm-1 in the 7Li case are obtained in the present work. In the 6 Li case a complete agreement between experiment and the calculated sum rule is found while in the 7Li case an agreement only at a qualitative level is observed.

  13. A method for investigation of the D(4He, γ)6Li reaction in the Ultralow energy region under a high background

    NASA Astrophysics Data System (ADS)

    Bystritsky, V. M.; Dudkin, G. N.; Krylov, A. R.; Gazi, S.; Huran, J.; Nechaev, B. A.; Padalko, V. N.; Sadovsky, A. B.; Tuleushev, Yu. Zh.; Filipowicz, M.; Philippov, A. V.

    2016-07-01

    The cosmological lithium problem, that is, a noticeable discrepancy between the predicted and observed abundances of lithium, is in conflict with the Standard Big Bang Nucleosynthesis model. For example, the abundance of 7Li is 2-4 times smaller than predicted by the Standard Big Bang Nucleosynthesis. As to the abundance of 6Li, recent more accurate optical investigations have yielded only the upper limit on the 6Li/7Li ratio, which makes the problem of 6Li abundance and accordingly of disagreement with the Standard Big Bang Nucleosynthesis predictions less acute. However, experimental study of the D(4He, γ)6Li reaction cross section is still of current importance because there is a theoretical approach predicting its anomalously large value in the region of energies below the Standard Big Bang Nucleosynthesis energy. The work is dedicated to the measurement of the cross section for the D(4He, γ)6Li reaction proceeding in zirconium deuteride at the incident 4He+ion energy of 36 keV. The experiment is performed at a pulsed Hall plasma accelerator with an energy spread of 20% FWHM. A method for direct measurement of the background from the reaction chain D(4He, 4He)D→D(D, n)3He→(n, γ) and/or (n, n‧γ) ending with activation of the surrounding material by neutrons is proposed and implemented in the work. An upper limit on the D(4He, γ)6Li reaction cross section σ≤7·10-36 cm2 at the 90% confidence level is obtained.

  14. New determination of 12C(α,γ)16O reaction rate

    NASA Astrophysics Data System (ADS)

    Oulebsir, N.

    2015-12-01

    The reaction 12C(α,γ)16O was investigated through the direct α-transfer reaction (7Li,t) at 28 and 34 MeV incident energies. We determined the reduced α-widths of the sub-threshold 2+ and 1- states of 16O from the DWBA analysis of the transfer reaction 12C(7Li,t)16O performed at two incident energies. The obtained result for the 2+ and 1- sub-threshold resonances as introduced in the R-matrix fitting of radiative capture and elastic-scattering data to determine the E2 and E1 S-factor from 0.01MeV to 4.2MeV in the center-of-mass energy. After determining the astrophysic factor of 12C(α,γ)16O S(E) with Pierre Descouvement code, I determined numerically the new reaction rate of this reaction at a different stellar temperature (0.06 Gk-2 GK). The 12C(α,γ)16O reaction rate at T9 = 0.2 is [7.21-2.25+2.15] × 10-15 cm3 s-1 mol-1. Some comparisons and discussions about our new 12C(α,γ)16O reaction rate are presented. The agreements of the reaction rate below T9 = 2 between our results and with those proposed by NACRE indicate that our results are reliable, and they could be included in the astrophysical reaction rate network.

  15. Anomalously High Isotope Ratio 3He/4He and Tritium in Deuterium-Loaded Metal: Evidence for Nuclear Reaction in Metal Hydrides at Low Temperature

    NASA Astrophysics Data System (ADS)

    Jiang, Song-Sheng; He, Ming; Wu, Shao-Yong; Qi, Bu-Jia

    2012-01-01

    Anomalous 3He/4He ratios in deuterium-loaded titanium samples are observed to be about 1-4 × 10-1, much greater than the values (<=10-4) in natural objects. Control experiments with the deuterium-unloaded titanium sample and original industrial deuterium gas are also carried out, but no anomalous 3He/4He values are observed. In addition, anomalous tritium in deuterium-loaded titanium samples are also observed. To explain the excess 3He and tritium in the deuterium-loaded titanium samples, it is required that the deuteron-induced nuclear reaction occurs in the samples at low temperature.

  16. Geometry and microwave rotational spectrum of the FC16O18O• radical.

    PubMed

    Koucký, Jan; Kania, Patrik; Uhlíková, Tereza; Kolesniková, Lucie; Beckers, Helmut; Willner, Helge; Urban, Stěpán

    2013-10-01

    The rotational spectrum of an asymmetrically substituted isotopologue of the fluoroformyloxyl radical FC(16)O(18)O(•) with resolved fine and hyperfine structures were measured and analyzed for the very first time. The molecular parameters of this radical obtained from the spectral analysis were processed along with the symmetrical isotopologues FC(16)O2(•) and FC(18)O2(•) and accurate substitution geometry was attained. In addition to those, coupled cluster quantum chemistry calculations were used to scale the experimental parameters, and in this manner, trustworthy values of the equilibrium and ground state geometries were derived.

  17. Spectral linelist of HD16O molecule based on VTT calculations for atmospheric application

    NASA Astrophysics Data System (ADS)

    Voronin, B. A.

    2014-11-01

    Three version line-list of dipole transition for isotopic modification of water molecule HD16O are presented. Line-lists have been created on the basis of VTT calculations (Voronin, Tennyson, Tolchenov et al. MNRAS, 2010) by adding air- and self-broadening coefficient, and temperature exponents for HD16O-air case. Three cut-of values for the line intensities were used: 1e-30, 1e-32 and 1e-35 cm/molecule. Calculated line-lists are available on the site ftp://ftp.iao.ru/pub/VTT/VTT-296/.

  18. Double Folding Potential of Different Interaction Models for 16O + 12C Elastic Scattering

    NASA Astrophysics Data System (ADS)

    Hamada, Sh.; Bondok, I.; Abdelmoatmed, M.

    2016-08-01

    The elastic scattering angular distributions for 16O + 12C nuclear system have been analyzed using double folding potential of different interaction models: CDM3Y1, CDM3Y6, DDM3Y1 and BDM3Y1. We have extracted the renormalization factor N r for the different concerned interaction models. Potential created by BDM3Y1 model of interaction has the shallowest depth which reflects the necessity to use higher renormalization factor. The experimental angular distributions for 16O + 12C nuclear system in the energy range 115.9-230 MeV exhibited unmistakable refractive features and rainbow phenomenon.

  19. Elastic {sup 16}O{sup 16}O scattering at E({sup 16}O) = 350 MeV and new method for a model-independent determination of the scattering matrix

    SciTech Connect

    Korda, V. Yu.; Molev, A. S.; Korda, L. P.

    2007-06-15

    A new approach that can be used to extract the scattering matrix S(l) as a complex-valued function of the orbital angular momentum l directly from experimental data on elastic nucleus-nucleus scattering at intermediate energies without resort to additional model assumptions is developed on the basis of the evolutionary algorithm. Owing to the fact that the behavior of the derivatives of S(l) is automatically monitored within this approach, the scattering matrix obtained for {sup 16}O{sup 16}O interaction at an energy of 350 MeV is determined by its absolute value and the nuclear phase shift, which are smooth monotonic functions of the orbital angular momentum. Moreover, the result involves no distortions, the form of the quantum deflection function being typical of the nuclear-rainbow pattern. It is shown that the ultimate form of S(l) is independent of input representations of the scattering matrix, which were usually taken on the basis of various phenomenological models.

  20. The 3H(d,γ)5He Reaction for Ec.m. ≤ 300 keV

    NASA Astrophysics Data System (ADS)

    Parker, C. E.; Brune, C. R.; Massey, T. N.; O'Donnell, J. E.; Richard, A. L.; Sayre, D. B.

    2016-03-01

    The 3H(d, γ)5He reaction has been measured using a 500-keV pulsed deuteron beam incident on a stopping titanium tritide target at Ohio University's Edwards Accelerator Laboratory. The time-of-flight (TOF) technique has been used to distinguish the γ-rays from neutrons detected in the bismuth germinate (BGO) γ-ray detector. A stilbene scintillator and an NE-213 scintillator have been used to detect the neutrons from the 3H(d, n)4He reaction using both the pulse-shape discrimination and TOF techniques. A newly-designed target holder with a silicon surface barrier detector to simultaneously measure α-particles to normalize the neutron count was incorporated for subsequent measurements. The γ-rays have been measured at laboratory angles of 0°, 45°, 90°, and 135°. Information about the γ-ray energy distribution for the unbound ground state and first excited state of 5He can be obtained experimentally by comparing the BGO data to Monte Carlo simulations. The 3H(d, γ)/3H(d, n) branching ratio has also been determined.

  1. Comparison of (/sup 3/H)nicotine and (/sup 3/H)acetylcholine binding in mouse brain: regional distribution

    SciTech Connect

    Sershen, H.; Reith, M.E.; Hashim, A.; Lajtha, A.

    1985-06-01

    In a continuing study of nicotine binding sites, the authors determined the relative amount of nicotine binding and acetylcholine binding in various brain regions of C57/BL and of DBA mice. Although midbrain showed the highest and cerebellum the lowest binding for both (/sup 3/H)nicotine and (/sup 3/H)acetylcholine, the ratio of nicotine to acetylcholine binding showed a three-fold regional variation. Acetylcholine inhibition of (/sup 3/H)nicotine binding indicated that a portion of nicotine binding was not inhibited by acetylcholine. These results indicate important differences between the binding of (+/-)-(/sup 3/H)nicotine and that of (/sup 3/H)acetylcholine.

  2. Angular correlation measurements for 4-{alpha} decaying states in {sup 16}O

    SciTech Connect

    Wuosmaa, A.H.; Back, B.B.; Betts, R.R.

    1995-08-01

    Previous measurements of the {sup 12}C({sup 12}C,{sup 8}Be){sup 16}O{sup *}(4 {alpha}) reaction identified discrete levels in {sup 16}O which decay by breakup into 4 {alpha} particles through a number of different decay sequences, including {sup 16}O{sup *} {yields} {sup 8}Be + {sup 8}Be and {alpha} + {sup 12}C (O{sub 2}{sup +}). These states are observed in a range of excitation energies where resonances are observed in inelastic {alpha} + {sup 12}C scattering leading to the {sup 8}Be + {sup 8}Be and {alpha} + {sup 12}C final states. These resonances were associated with 4 {alpha}-particle chain configurations in {sup 16}O. Should the states populated in the {sup 12}C + {sup 12}C reaction possess this same extended structure, it would serve as an important piece of evidence supporting the idea that even more deformed structures are formed in the {sup 24}Mg compound system. In order to more firmly make this association, it is important to determine the spins of the states populated in the {sup 12}C + {sup 12}C reaction.

  3. Evidence for a Long Duration of the 16O-Rich Reservoir in the Solar Nebula

    NASA Astrophysics Data System (ADS)

    Ushikubo, T.; Tenner, T. J.; Hiyagon, H.; Kita, N. T.

    2016-08-01

    Oxygen isotope ratios and 26Al-26Mg systematics of a pyroxene-anorthite-rich CAI from Acfer 094 suggest decomposition of melilite occurred in an 16O-rich environment at ~2.3 million years after normal CAI formation.

  4. Probing the Repulsive Core of the Nucleon-Nucleon Interaction via the 4He(e,e`pN) Triple-Coincidence Reaction

    DOE PAGES

    Korover, Igor; Muangma, Navaphon; Hen, Or; Shneor, Ran; Sulkosky, Vincent; Kelleher, Aidan; Gilad, Shalev; Higinbotham, Douglas; Piasetzky, Eliazer; Wood, Stephen; et al

    2014-07-01

    We studied simultaneously the 4He(e,e'p), 4He(e,e'pp), and 4He(e,e'pn) reactions at Q2=2 [GeV/c]2 and xB >1, for a (e,e'p) missing-momentum range of 400 to 830 MeV/c. The knocked-out proton was detected in coincidence with a proton or neutron recoiling almost back to back to the missing momentum, leaving the residual A=2 system at low excitation energy. These data were used to identify two-nucleon short-range correlated pairs and to deduce their isospin structure as a function of missing momentum in a region where the nucleon-nucleon force is expected to change from predominantly tensor to repulsive. Neutron-proton pairs dominate the high-momentum tail ofmore » the nucleon momentum distributions, but their abundance is reduced as the nucleon momentum increases beyond ~500 MeV/c. The extracted fraction of proton-proton pairs is small and almost independent of the missing momentum in the range we studied. Our data are compared with ab-initio calculations of two-nucleon momentum distributions in 4He.« less

  5. Search for the enhancement of the thermal expansion coefficient of superfluid 4HE Near T_Lambada by a heat current

    NASA Technical Reports Server (NTRS)

    Liu, Y.; Israelsson, U.; Larson, M.

    2001-01-01

    Presentation on the transition in 4He in the presence of a heat current (Q) provides an ideal system for the study of phase transitions under non-equlibrium, dynamical conditions. Many physical properties become nonlinear and Q-dependant near the transition temperature, T_Lambada.

  6. Rapid and convenient preparation of (4-/sup 3/H)NADP and stereospecifically tritiated NADP/sup 3/H

    SciTech Connect

    Moran, R.G.; Sartori, P.; Reich, V.

    1984-04-01

    The enzymatic preparation and chromatographic purification of (4-/sup 3/H)NADP and NADPH stereospecifically labeled with /sup 3/H on either the A or B faces at position 4 have been simplified. Commercially available (1-/sup 3/H)glucose was used as a starting material for the sequential synthesis of (4B-/sup 3/H)NADPH, (4-/sup 3/H)NADP, and (4A-/sup 3/H)NADPH. These products were rapidly purified by step elution of DEAE-cellulose minicolumns so that (4B-/sup 3/H)NADPH was produced and purified from (1-/sup 3/H)glucose in 2 h, (4-/sup 3/H)NADP in 5 h, and (4A-/sup 3/H)NADPH in 8 h. Yields of these products were 65 to 88% starting with (1-/sup 3/H)glucose. Analysis of the products by high-performance liquid chromatography indicated radiochemical purities of 82-95% for these compounds and specific activities equivalent to that of the starting material (10-15 Ci/mmol). 15 references.

  7. Total cross section of the 3H(p,n)3He reaction from threshold to 4.5 MeV

    NASA Astrophysics Data System (ADS)

    Brune, C. R.; Hahn, K. I.; Kavanagh, R. W.; Wrean, P. R.

    1999-07-01

    We report new measurements of the total cross section for the 3H(p,n)3He reaction from threshold (Ep=1.02 MeV) to Ep=4.5 MeV. The experiment utilized specially prepared Ti-3H targets, and neutrons were detected using a 4π detector. A weak resonant structure due to an excited state in 4He is observed which was not seen in previous cross section measurements. A new expression for the 3He(n,p)3H thermonuclear reaction rate for temperatures below 10 GK is presented which will allow for more accurate calculations of the yields of light elements produced by big-bang nucleosynthesis.

  8. A comparison of groundwater dating with 81Kr, 36Cl and 4He in four wells of the Great Artesian Basin, Australia

    NASA Astrophysics Data System (ADS)

    Lehmann, B. E.; Love, A.; Purtschert, R.; Collon, P.; Loosli, H. H.; Kutschera, W.; Beyerle, U.; Aeschbach-Hertig, W.; Kipfer, R.; Frape, S. K.; Herczeg, A.; Moran, J.; Tolstikhin, I. N.; Gröning, M.

    2003-06-01

    The isotopic ratios 81Kr/Kr and 36Cl/Cl and the 4He concentrations measured in groundwater from four artesian wells in the western part of the Great Artesian Basin (GAB) in Australia are discussed. Based on radioactive decay along a water flow path the 81Kr/Kr ratios are directly converted to groundwater residence times. Results are in a range of 225-400 kyr with error bars in the order of 15% primarily due to counting statistics in the cyclotron accelerator mass spectrometer measurement. Additional uncertainties from subsurface production and/or exchange with stagnant porewaters in the confining shales appear to be of the same order of magnitude. These 81Kr ages are then used to calibrate the 36Cl and the 4He dating methods. Based on elemental analyses of rock samples from the sandstone aquifer as well as from the confining Bulldog shale the in situ flux of thermal neutrons and the corresponding 3He/ 4He and 36Cl/Cl ratios are calculated. From a comparison of: (i) the 3He/ 4He ratios measured in the groundwater samples with the calculated in situ ratios in rocks and (ii) the measured δ 37Cl ratios with the 4He concentrations measured in groundwater it is concluded that both helium and chloride are most likely added to the aquifer from sources in the stagnant porewaters of the confining shale by diffusion and/or mixing. Based on this 'working hypothesis' the 36Cl transport equation in groundwater is solved taking into account: (i) radioactive decay, (ii) subsurface production in the sandstone aquifer (with an in situ 36Cl/Cl ratio of 6×10 -15) and (iii) addition of chloride from a source in the confining shale (with a 36Cl/Cl ratio of 13×10 -15). Lacking better information it is assumed that the chloride concentration increased linearly with time from an (unknown) initial value Ci to its measured present value C= Ci+ Ca, where Ca represents the (unknown) amount of chloride added from subsurface sources. Using the 81Kr ages of the four groundwater samples and a

  9. Determination of the delta(18O/16O)of Water: RSIL Lab Code 489

    USGS Publications Warehouse

    Revesz, Kinga; Coplen, Tyler

    2008-01-01

    The purpose of the technique described by the Reston Stable Isotope Laboratory (RSIL) lab code 489 is to present a method to determine the delta(180/160), abbreviated as delta-180, of water. This delta-18O measurement of water also is a component of National Water Quality Laboratory (NWQL in USGS) schedules 1142 and 1172. Water samples are loaded into glass sample containers on a vacuum manifold to equilibrate gaseous CO2 at constant temperature (25 deg C) with water samples. After loading water samples on the vacuum manifold, air is evacuated through capillary to avoid evaporation, and CO2 is added. The samples are shaken to increase the equilibration rate of water and CO2. When isotopic equilibrium has been attained, an aliquot of CO2 is extracted sequentially from each sample container, separated from water vapor by means of a dry ice trap, and introduced into a dual-inlet isotope-ratio mass spectrometer (DI-IRMS) for determination of the delta-18O value. There is oxygen isotopic fractionation between water and CO2, but it is constant at constant temperature. The DI-IRMS is a DuPont double-focusing mass spectrometer. It has a double collector. One ion beam passes through a slit in a forward collector and is collected in the rear collector. The other ion beams are collected in the front collector. The instrument is capable of measuring mass/charge (m/z) 44 and 45 or 44 and 46 by changing the ion-accelerating voltage under computer control. The ion beams from these m/z values are as follows: m/z 44=CO2=12C16O16O, m/z 45=CO2=13C16O16O primarily, and m/z 46 = CO2=12C16O18O primarily. The data acquisition and control software calculates delta-18O values.

  10. Large and unexpected enrichment in stratospheric 16O13C18O and its meridional variation.

    PubMed

    Yeung, Laurence Y; Affek, Hagit P; Hoag, Katherine J; Guo, Weifu; Wiegel, Aaron A; Atlas, Elliot L; Schauffler, Sue M; Okumura, Mitchio; Boering, Kristie A; Eiler, John M

    2009-07-14

    The stratospheric CO(2) oxygen isotope budget is thought to be governed primarily by the O((1)D)+CO(2) isotope exchange reaction. However, there is increasing evidence that other important physical processes may be occurring that standard isotopic tools have been unable to identify. Measuring the distribution of the exceedingly rare CO(2) isotopologue (16)O(13)C(18)O, in concert with (18)O and (17)O abundances, provides sensitivities to these additional processes and, thus, is a valuable test of current models. We identify a large and unexpected meridional variation in stratospheric (16)O(13)C(18)O, observed as proportions in the polar vortex that are higher than in any naturally derived CO(2) sample to date. We show, through photochemical experiments, that lower (16)O(13)C(18)O proportions observed in the midlatitudes are determined primarily by the O((1)D)+CO(2) isotope exchange reaction, which promotes a stochastic isotopologue distribution. In contrast, higher (16)O(13)C(18)O proportions in the polar vortex show correlations with long-lived stratospheric tracer and bulk isotope abundances opposite to those observed at midlatitudes and, thus, opposite to those easily explained by O((1)D)+CO(2). We believe the most plausible explanation for this meridional variation is either an unrecognized isotopic fractionation associated with the mesospheric photochemistry of CO(2) or temperature-dependent isotopic exchange on polar stratospheric clouds. Unraveling the ultimate source of stratospheric (16)O(13)C(18)O enrichments may impose additional isotopic constraints on biosphere-atmosphere carbon exchange, biosphere productivity, and their respective responses to climate change.

  11. High performance cobalt-free Cu1.4Mn1.6O4 spinel oxide as an intermediate temperature solid oxide fuel cell cathode

    NASA Astrophysics Data System (ADS)

    Zhen, Shuying; Sun, Wang; Li, Peiqian; Tang, Guangze; Rooney, David; Sun, Kening; Ma, Xinxin

    2016-05-01

    In this work Cu1.4Mn1.6O4 (CMO) spinel oxide is prepared and evaluated as a novel cobalt-free cathode for intermediate temperature solid oxide fuel cells (IT-SOFCs). Single phase CMO powder with cubic structure is identified using XRD. XPS results confirm that mixed Cu+/Cu2+ and Mn3+/Mn4+ couples exist in the CMO sample, and a maximum conductivity of 78 S cm-1 is achieved at 800 °C. Meanwhile, CMO oxide shows good thermal and chemical compatibility with a 10 mol% Sc2O3 stabilized ZrO2 (ScSZ) electrolyte material. Impedance spectroscopy measurements reveals that CMO exhibits a low polarization resistance of 0.143 Ω cm2 at 800 °C. Furthermore, a Ni-ScSZ/ScSZ/CMO single cell demonstrates a maximum power density of 1076 mW cm-2 at 800 °C under H2 (3% H2O) as the fuel and ambient air as the oxidant. These results indicate that Cu1.4Mn1.6O4 is a superior and promising cathode material for IT-SOFCs.

  12. Fractionation of Oxygen Isotopes by Thermal Ionization Mass Spectrometry Inferred from Simultaneous Measurement of (17)O/(16)O and (18)O/(16)O Ratios and Implications for the (182)Hf-(182)W Systematics.

    PubMed

    Trinquier, Anne

    2016-06-01

    Accurate (182)Hf-(182)W chronology of early planetary differentiation relies on highly precise and accurate tungsten isotope measurements. WO3(-) analysis by negative thermal ionization mass spectrometry requires W(17)O(16)O2(-), W(17)O2(16)O(-), W(18)O(16)O2(-), W(17)O3(-), W(17)O(18)O(16)O(-), and W(18)O2(16)O(-) isotopologue interference corrections on W(16)O3(-) species ( Harper et al. Geochim. Cosmochim. Acta 1996 , 60 , 1131 ; Quitté et al. Geostandard. Newslett. 2002 , 26 , 149 ; Trinquier et al. Anal. Chem. 2016 , 88 , 1542 ; Touboul et al. Nature 2015 , 520 , 530 ; Touboul et al. Int. J. Mass Spectrom. 2012 , 309 , 109 ). In addition, low ion beam intensity counting statistics combined with Faraday cup detection noise limit the precision on the determination of (18)O/(16)O and (17)O/(16)O relative abundances. Mass dependent variability of (18)O/(16)O over the course of an analysis and between different analyses calls for oxide interference correction on a per integration basis, based on the in-run monitoring of the (18)O/(16)O ratio ( Harper et al. Geochim. Cosmochim. Acta 1996 , 60 , 1131 ; Quitté et al. Geostandard. Newslett. 2002 , 26 , 149 ; Trinquier et al. Anal. Chem. 2016 , 88 , 1542 ). Yet, the (17)O/(16)O variation is normally not being monitored and, instead, inferred from the measured (18)O/(16)O variation, assuming a δ(17)O-δ(18)O Terrestrial Fractionation Line ( Trinquier et al. Anal. Chem. 2016 , 88 , 1542 ). The purpose of the present study is to verify the validity of this assumption. Using high resistivity amplifiers, (238)U(17)O2 and (238)U(18)O2 ion beams down to 1.6 fA have been monitored simultaneously with (235,238)U(16)O2 species in a uranium certified reference material. This leads to a characterization of O isotope fractionation by thermal ionization mass spectrometry in variable loading and running conditions (additive-to-sample ratio, PO2 pressure, presence of ionized metal and oxide species). Proper determination of O

  13. Fractionation of Oxygen Isotopes by Thermal Ionization Mass Spectrometry Inferred from Simultaneous Measurement of (17)O/(16)O and (18)O/(16)O Ratios and Implications for the (182)Hf-(182)W Systematics.

    PubMed

    Trinquier, Anne

    2016-06-01

    Accurate (182)Hf-(182)W chronology of early planetary differentiation relies on highly precise and accurate tungsten isotope measurements. WO3(-) analysis by negative thermal ionization mass spectrometry requires W(17)O(16)O2(-), W(17)O2(16)O(-), W(18)O(16)O2(-), W(17)O3(-), W(17)O(18)O(16)O(-), and W(18)O2(16)O(-) isotopologue interference corrections on W(16)O3(-) species ( Harper et al. Geochim. Cosmochim. Acta 1996 , 60 , 1131 ; Quitté et al. Geostandard. Newslett. 2002 , 26 , 149 ; Trinquier et al. Anal. Chem. 2016 , 88 , 1542 ; Touboul et al. Nature 2015 , 520 , 530 ; Touboul et al. Int. J. Mass Spectrom. 2012 , 309 , 109 ). In addition, low ion beam intensity counting statistics combined with Faraday cup detection noise limit the precision on the determination of (18)O/(16)O and (17)O/(16)O relative abundances. Mass dependent variability of (18)O/(16)O over the course of an analysis and between different analyses calls for oxide interference correction on a per integration basis, based on the in-run monitoring of the (18)O/(16)O ratio ( Harper et al. Geochim. Cosmochim. Acta 1996 , 60 , 1131 ; Quitté et al. Geostandard. Newslett. 2002 , 26 , 149 ; Trinquier et al. Anal. Chem. 2016 , 88 , 1542 ). Yet, the (17)O/(16)O variation is normally not being monitored and, instead, inferred from the measured (18)O/(16)O variation, assuming a δ(17)O-δ(18)O Terrestrial Fractionation Line ( Trinquier et al. Anal. Chem. 2016 , 88 , 1542 ). The purpose of the present study is to verify the validity of this assumption. Using high resistivity amplifiers, (238)U(17)O2 and (238)U(18)O2 ion beams down to 1.6 fA have been monitored simultaneously with (235,238)U(16)O2 species in a uranium certified reference material. This leads to a characterization of O isotope fractionation by thermal ionization mass spectrometry in variable loading and running conditions (additive-to-sample ratio, PO2 pressure, presence of ionized metal and oxide species). Proper determination of O

  14. Measurement of the isotopic ratio distribution of HD16O and H2 16O in the 20-38 km altitude range from far-infrared spectra

    NASA Astrophysics Data System (ADS)

    Dinelli, Bianca Maria; Lepri, Gianmarco; Carlotti, Massimo; Carli, Bruno; Mencaraglia, Francesco; Ridolfi, Marco; Nolt, Ira G.; Ade, Peter A. R.

    1997-08-01

    The altitude distribution of the isotopic ratio between HD16O and H216O in the stratosphere is derived by retrieving the mixing ratio profiles (from 20 km to 38 km of altitude) of the two isotopic species from far-infrared emission spectra. The measurements were made with a balloon-borne Fourier Transform Spectrometer capable of 0.0025 cm-1 spectral resolution during the IBEX 92 campaign. The retrievals were carried out using the global-fit procedure on a statistically significant number of spectra for each isotope, in the 40-75 cm-1 spectral region. This measurement determines the D/H ratio in stratospheric water over an altitude range larger than that of previous measurements. The value of the HD16O/H216O ratio, normalized to the standard value, ranges from 0.4 to 0.5 (with a 10% random error) in the altitude range studied and is in good agreement with the values previously measured.

  15. Elastic scattering of {sup 16}O+{sup 16}O at energies E/A between 5 and 8 MeV

    SciTech Connect

    Nicoli, M. P.; Haas, F.; Freeman, R. M.; Aissaoui, N.; Beck, C.; Elanique, A.; Nouicer, R.; Morsad, A.; Szilner, S.; Basrak, Z.

    1999-12-01

    The elastic scattering of {sup 16}O+{sup 16}O has been measured at nine energies between E{sub lab}=75 and 124 MeV. The data cover up to 100 degree sign in the c.m. and can be described in terms of phenomenological and folding model potentials which reproduce the main features observed. In agreement with studies at higher energies in this and similar systems, refractive effects are present in the angular distributions at all energies. In particular, the passage of Airy minima through 90 degree sign at E{sub c.m.}=40, 47.5, and 62 MeV explains the deep minima observed in the excitation function. The real part of the optical potential is found to vary very little with energy over the studied interval, but the imaginary part shows a rapid change in its shape at incident energy about 90 MeV. Nonetheless, the energy dependence of the volume integral of the real and imaginary parts is in agreement with dispersion relation predictions. (c) 1999 The American Physical Society.

  16. Synthesis and characterization of 3H-labelled tetrahydrobiopterin.

    PubMed Central

    Werner, E R; Schmid, M; Werner-Felmayer, G; Mayer, B; Wachter, H

    1994-01-01

    We synthesized [3'-3H]-5,6,7,8-tetrahydrobiopterin from [8,5'-3H]guanosine 5'-triphosphate ([8,5'-3H]GTP) using GTP cyclohydrolase (EC 3.5.4.16), 6-pyruvoyltetrahydropterin synthase and sepiapterin reductase (EC 1.1.1.153). After purification by cation-exchange h.p.l.c. a solution of radiochemically pure (> 95%) [3'-3H]-5,6,7,8-tetrahydrobiopterin with a specific activity of 9.2 Ci/mmol was obtained. The product proved well suited for studying the binding of tetrahydrobiopterin to nitric-oxide synthase. PMID:7528005

  17. Partial chemical characterization of cyclopyrrolones ((/sup 3/H) suriclone) and benzodiazepines ((/sup 3/H)flunitrazepam) binding site: Differences

    SciTech Connect

    Zundel, J.L.; Blanchard, J.C.; Julou, L.

    1985-06-10

    Rat hippocampus membranes were treated with several protein modifying reagents (iodoacetamide, N-ethylmaleimide, tetranitromethane and N-acetylimidazole). The effects of these treatments on the binding sites of cyclopyrrolones ((/sup 3/H) suriclone), a new chemical family of minor tranquilizers, and benzodiazepines ((/sup 3/H) flunitrazepam) were investigated. Here the authors show that both ligands are similarly sensitive to cysteine alkylation: (/sup 3/H) suriclone and (/sup 3/H) flunitrazepam binding are reduced by iodoacetamide and slightly increased by N-ethylmaleimide. On the contrary they are clearly differentiated by tyrosine modification: (/sup 3/H) suriclone binding is not changed whereas (/sup 3/H) flunitrazepam binding is increased by tetranitromethane and decreased by N-acetylimidazole. The present findings and published evidence suggest cyclopyrrolones and benzodiazepines bind to distinct sites or to different allosteric forms of the benzodiazepine receptor. 28 references, 6 figures.

  18. 186Os and 187Os enrichments and high-3He/4He sources in the Earth’s mantle: Evidence from Icelandic picrites

    NASA Astrophysics Data System (ADS)

    Brandon, Alan D.; Graham, David W.; Waight, Tod; Gautason, Bjarni

    2007-09-01

    Picrites from the neovolcanic zones in Iceland display a range in 187Os/ 188Os from 0.1297 to 0.1381 (γ Os = + 2.1 to +8.7) and uniform 186Os/ 188Os of 0.1198375 ± 32 (2 σ). The value for 186Os/ 188Os is within uncertainty of the present-day value for the primitive upper mantle of 0.1198398 ± 16. These Os isotope systematics are best explained by ancient recycled crust or melt enrichment in the mantle source region. If so, then the coupled enrichments displayed in 186Os/ 188Os and 187Os/ 188Os from lavas of other plume systems must result from an independent process, the most viable candidate at present remains core-mantle interaction. While some plumes with high 3He/ 4He, such as Hawaii, appear to have been subjected to detectable addition of Os (and possibly He) from the outer core, others such as Iceland do not. A positive correlation between 187Os/ 188Os and 3He/ 4He from 9.6 to 19 Ra in Iceland picrites is best modeled as mixtures of 1 Ga or older ancient recycled crust mixed with primitive mantle or incompletely degassed depleted mantle isolated since 1-1.5 Ga, which preserves the high 3He/ 4He of the depleted mantle at the time. These mixtures create a hybrid source region that subsequently mixes with the present-day convecting MORB mantle during ascent and melting. This multistage mixing scenario requires convective isolation in the deep mantle for hundreds of million years or more to maintain these compositionally distinct hybrid sources. The 3He/ 4He of lavas derived from the Iceland plume changed over time, from a maximum of 50 Ra at 60 Ma, to approximately 25-27 Ra at present. The changes are coupled with distinct compositional gaps between the different aged lavas when 3He/ 4He is plotted versus various geochemical parameters such as 143Nd/ 144Nd and La/Sm. These relationships can be interpreted as an increase in the proportion of ancient recycled crust in the upwelling plume over this time period. The positive correlation between 187Os/ 188Os and

  19. Asthenosphere-lithosphere interactions in Western Saudi Arabia: Inferences from 3He/4He in xenoliths and lava flows from Harrat Hutaymah

    NASA Astrophysics Data System (ADS)

    Konrad, Kevin; Graham, David W.; Thornber, Carl R.; Duncan, Robert A.; Kent, Adam J. R.; Al-Amri, Abdullah M.

    2016-04-01

    Extensive volcanic fields on the western Arabian Plate have erupted intermittently over the last 30 Ma following emplacement of the Afar flood basalts in Ethiopia. In an effort to better understand the origin of this volcanism in western Saudi Arabia, we analyzed 3He/4He, and He, CO2 and trace element concentrations in minerals separated from xenoliths and lava flows from Harrat Hutaymah, supplemented with reconnaissance He isotope data from several other volcanic fields (Harrat Al Birk, Harrat Al Kishb and Harrat Ithnayn). Harrat Hutaymah is young (< 850 ka) and the northeasternmost of the volcanic fields. There is a remarkable homogeneity of 3He/4He trapped within most xenoliths, with a weighted mean of 7.54 ± 0.03 RA (2σ, n = 20). This homogeneity occurs over at least eight different xenolith types (including spinel lherzolite, amphibole clinopyroxenite, olivine websterite, clinopyroxenite and garnet websterite), and encompasses ten different volcanic centers within an area of ~ 2500 km2. The homogeneity is caused by volatile equilibration between the xenoliths and fluids derived from their host magma, as fluid inclusions are annealed during the infiltration of vapor-saturated magmas along crystalline grain boundaries. The notable exceptions are the anhydrous spinel lherzolites, which have a lower weighted mean 3He/4He of 6.8 ± 0.3 RA (2σ, n = 2), contain lower concentrations of trapped He, and have a distinctly depleted light rare earth element signature. 3He/4He values of ~ 6.8 RA are also commonly found in spinel lherzolites from harrats Ithnayn, Al Birk, and from Zabargad Island in the Red Sea. Olivine from non-xenolith-bearing lava flows at Hutaymah spans the He isotope range of the xenoliths. The lower 3He/4He in the anhydrous spinel lherzolites appears to be tied to remnant Proterozoic lithosphere prior to metasomatic fluid overprinting. Elevated 3He/4He in the western harrats has been observed only at Rahat (up to 11.8 RA; Murcia et al., 2013), a

  20. Radiotoxicities of (/sup 3/H)thymidine and of (/sup 3/H)arginine compared in mouse embryos in vitro

    SciTech Connect

    Mueller, W.U.S.; Streffer, C.; Molls, M.; Glueck, L.

    1987-05-01

    Tritium that is bound to organic molecules is of special risk for living systems, in particular when such molecules are components of the cell nucleus. Therefore, (/sup 3/H)thymidine and (/sup 3/H)arginine were studied for radiotoxicity in early mammalian embryo development. Starting with the two-cell stage, mouse embryos were incubated in vitro with (/sup 3/H)thymidine or (/sup 3/H)arginine at either 370 Bq/ml (10 nCi/ml) or 925 Bq/ml (25 nCi/ml). Development in vitro was followed up to the formation of the inner cell mass at 192 h postconception (p.c.). There was no difference in radiotoxicity of the two substances with respect to cell proliferation; however, formation of blastocysts, hatching of blastocysts, trophoblast outgrowth, and formation of inner cell mass were impaired more strongly by (/sup 3/H)arginine than by (/sup 3/H)thymidine when the external exposure concentrations were the same. Similarly, micronuclei were seen in blastocysts at 96 h p.c. at higher frequency after incubation with (/sup 3/H)arginine. However, uptake of (/sup 3/H)arginine by the embryos was considerably faster than that of (/sup 3/H)thymidine, and this most probably accounts for the apparent difference in radiotoxicity.

  1. Parkinson's disease: decreased density of /sup 3/H-imipramine and /sup 3/H-paroxetine binding sites in putamen

    SciTech Connect

    Raisman, R.; Cash, R.; Agid, Y.

    1986-04-01

    The density of high-affinity /sup 3/H-imipramine and /sup 3/H-paroxetine binding sites (two serotonin-uptake blockers) was decreased in the putamen of parkinsonian patients. The correlation between serotonin levels and the number of /sup 3/H-imipramine and /sup 3/H-paroxetine binding sites suggests that they are located on serotoninergic nerve terminals and could be used to study serotoninergic innervation in the human brain. Since imipramine and paroxetine are powerful antidepressants, these results furthermore suggest that decreased serotoninergic transmission may be implicated in the pathophysiology of depression in Parkinson's disease.

  2. Comparison of ( sup 3 H)Phencyclidine (( sup 3 H)PCP) and ( sup 3 H) N-(1-(2-thienyl) cyclohexyl)piperidine (( sup 3 H)TCP) binding properties to rat and human brain membranes

    SciTech Connect

    Vignon, J.; Chaudieu, I.; Allaoua, H.; Journod, L.; Javoy-Agid, F.; Agid, Y.; Chicheportiche, R.

    1989-01-01

    The investigation of ({sup 3}H)PCP and ({sup 3}H)TCP binding properties to rat cerebrum and cerebellum resulted in the demonstration of multiple binding sites for the two drugs. In the two tissue preparations PCP had a lower affinity than TCP. In membranes from the cerebrum an equal number of high affinity binding sites were present for ({sup 3}H)PCP and ({sup 3}H)TCP. However, low affinity binding sites were two times more numerous for ({sup 3}H)PCP than for ({sup 3}H)TCP. In the cerebellum, the number of high and low affinity sites labeled by the two radioligands was identical, but the number of high affinity sites was about 7 fold lower than in cerebrum. In human cerebral cortex samples ({sup 3}H)TCP also bound to two different sites. The number of high and low affinity sites were 12 and 3 times, respectively, less abundant than in the rat cerebrum. Low affinity sites were of higher affinity than corresponding sites in the rat brain. In the human cerebellum ({sup 3}H)TCP binding parameters were identical to those measured in the same region in the rat.

  3. Analogs of the giant dipole and spin-dipole resonances in {sup 4}He and in {alpha} clusters of {sup 6,7}Li studied by the {sup 4}He,{sup 6,7}Li({sup 7}Li,{sup 7}Be{gamma}) reactions

    SciTech Connect

    Nakayama, S.; Matsumoto, E.; Fushimi, K.; Hayami, R.; Kawasuso, H.; Yasuda, K.; Yamagata, T.; Akimune, H.; Ikemizu, H.; Asaji, S.; Ishida, T.; Kudoh, T.; Sagara, K.; Fujiwara, M.; Hashimoto, H.; Kawase, K.; Nakanishi, K.; Oota, T.; Yosoi, M.; Greenfield, M. B.

    2008-07-15

    We studied analogs of the giant dipole resonance (GDR) and spin-dipole resonance (SDR) in {sup 4}He and in the {alpha} clusters of {sup 6,7}Li via the ({sup 7}Li,{sup 7}Be{gamma}) reactions on {sup 4}He, {sup 6}Li, and {sup 7}Li at an incident energy of 455 MeV and at a scattering angle of 0 deg. by measuring spin-nonflip and spin-flip spectra. The reaction Q-values for the analogs of the GDR and SDR in the {alpha} clusters of {sup 6,7}Li were found to be more negative than those in {sup 4}He by 2.0{+-}0.5 MeV. The ratios of the cross section for the analog of the GDR to that for the analog of the SDR in {sup 4}He and in the {alpha} clusters of {sup 6}Li and {sup 7}Li were found to be the same within errors, 0.5{+-}0.1. The cross sections for the analogs of the GDR as well as those for the analogs of the SDR in the {alpha} clusters of {sup 6,7}Li were 0.6{approx}0.8 times smaller than those in {sup 4}He. These results suggest that excitations of {alpha} clusters embedded in nuclei are suppressed as compared with excitations of free {alpha} particles.

  4. Two-neutron stripping in ({sup 18}O, {sup 16}O) and (t,p) reactions

    SciTech Connect

    Cavallaro, M.; Agodi, A.; Carbone, D.; Cunsolo, A.; Bondì, M.; Cappuzzello, F.; Nicolosi, D.; Tropea, S.; Borello-Lewin, T.; Rodrigues, M. R. D.; De Napoli, M.; Garcia, V. N.

    2014-11-11

    The {sup 12}C({sup 18}O,{sup 16}O){sup 14}C reactions has been investigated at 84 MeV incident energy. The charged ejectiles produced in the reaction have been momentum analyzed and identified by the MAGNEX magnetic spectrometer. Q-value spectra have been extracted with an energy resolution of 160 keV (Full Width at Half Maximum) and several known bound and resonant states of {sup 14}C have been identified up to 15 MeV. In particular, excited states with dominant 2p - 4h configuration are the most populated. The absolute values of the cross sections have been extracted showing a striking similarity with those measured for the same transitions by (t,p) reactions. This indicates that the effect of the {sup 16}O core is negligible in the reaction mechanism.

  5. One-two step transfer observed in 16O+11B nuclear system

    NASA Astrophysics Data System (ADS)

    Hamada, Sh.; Burtebayev, N.

    2015-06-01

    The angular distribution measurements for 16O ion beam elastically scattered from 11B target of thickness 32.9μg/cm2 at energy 22.4 MeV had been performed in the cyclotron DC-60 INP NNC RK. The previous measurements for 16O+11B nuclear system at energies 27, 30, 32.5 and 35 MeV showed an increase in the differential cross-section at backward angles due to the contribution of cluster transfer. Such transfer process could not be described in terms of optical model (OM); it could be described within the framework of distorted wave Born approximation method implemented in FRESCO code. Both one (5Li) and two-step transfer (proton transfer followed by Alpha transfer) were taken into considerations. We have extracted the spectroscopic amplitude (SA) for the configuration 16O→11B+5Li.

  6. Isotopic diversity in interplanetary dust particles and preservation of extreme 16O-depletion

    NASA Astrophysics Data System (ADS)

    Starkey, N. A.; Franchi, I. A.; Lee, M. R.

    2014-10-01

    Two interplanetary dust particles (IDPs) investigated by NanoSIMS reveal diverse oxygen isotope compositions at the micrometre-scale. The oxygen isotope values recorded at different locations across the single IDP fragments cover a wider range than the bulk values available from all IDPs and bulk meteorites measured to date. Measurement of H, C, and N isotopes by NanoSIMS, and the use of scanning and transmission electron microscopy (SEM and TEM) to determine elemental compositions and textural information allows for a better understanding of the lithologies and organic signatures associated with the oxygen isotope features. IDP Balmoral, a ∼15 μm-sized fragment with a chondritic porous (CP)-IDP-like texture, contains a region a few micrometres in size characterised by 16O-depleted isotope signatures in the range δ17O, δ18O = +80‰ to +200‰. The remainder of the fragment has a more 16O-rich composition (δ18O = 0-20‰), similar to many other IDPs and bulk meteorites. Other than in discrete pre-solar grains, such extreme 16O-depletions have only been observed previously in rare components within the matrix of the Acfer 094 meteorite. However, TEM imaging and FeO/MgO/Si ion ratios indicate that the 16O-depleted regions in Balmoral did not form by the same mechanism as that proposed for the 16O-depleted phases in Acfer 094. As the level of 16O depletion is consistent with that expected from isotope selective self-shielding, it is likely that the 16O-depleted reservoir was located close to that where oxygen self-shielding effects were most pronounced (i.e., the outer solar nebula or even interstellar medium). Individual regions within IDP Lumley cover a range in δ18O from -30‰ to +19‰, with the oxygen isotope values broadly co-varying with δD, δ13C, δ15N, light-element ratios and texture. The relationships observed in Lumley indicate that the parent body incorporated material at the micrometre-scale from discrete diverse isotopic reservoirs, some of

  7. Autoradiographic analysis of 3H-glutamate, 3H-dopamine, and 3H-GABA accumulation in rabbit retina after kainic acid treatment

    SciTech Connect

    Hampton, C.K.; Redburn, D.A.

    1983-01-01

    We have previously reported that exposure of isolated rabbit retina to 10(-3) M kainic acid produces profound morphological changes in specific retinal neurons (Hampton et al, 1981). We noted specific swelling of horizontal cell bodies and neurites, necrosis of cell bodies in the amacrine and ganglion cell layers, and swelling of elements in the inner plexiform layer. We now report a differential sensitivity to kainic acid of specific subclasses of amacrine cells autoradiographically labeled with 3H-glutamate, 3H-GABA, or 3H-dopamine. Three different effects were observed: (1) Labeling of neurons after incubation in 3H-glutamate was uniformly reduced while labeling of glia was much less affected. (2) The accumulation of 3H-dopamine was also decreased by kainic acid in two of the three labeled bands of the inner plexiform layer. The outermost labeled band was insensitive to kainic acid at the highest concentration tested (10(-2) M). These findings provide a basis for the subclassification of dopaminergic amacrine cells into at least two subclasses based on their sensitivity to kainic acid. (3) Kainic acid caused a dramatic increase in the labeling of GABAergic amacrine cell bodies and their terminals. This increased intensity may reflect a compensatory increase in uptake activity in response to kainic acid-induced depletion of endogenous GABA stores. These results confirm the highly toxic nature of kainic acid and demonstrate a high degree of specificity and complexity in its action in the retina.

  8. Factors influencing the 18O/16O-ratio in meat juices.

    PubMed

    Thiem, Ines; Lüpke, Matthias; Seifert, Hermann

    2004-09-01

    With respect to the question of whether the 18O/16O-ratio of meat water could be used for meat origin analysis, factors influencing its delta18O-value have been examined. The 18O/16O-ratio of meat water differs geographically, similar to known differences in precipitation and ground water. In Great Britain higher enrichments in 18O were found in southern samples and in Germany in northern samples. However, it was not possible to distinguish between British and German beef: their 18O/16O-ratios overlapped. British bovine samples the variation range of delta18O-values was 2.8 per thousand; in porcine samples it was 2.0 per thousand. British meat liquids from beef were enriched in 18O by 1.3 +/- 0.3 per thousand compared with pork. In porcine samples of litter mates with identical breeding and age at slaughter, the range in the delta18O-values among individuals was 2.4 per thousand. Experiments revealed significant influences of the meat's storage and handling conditions on the 18O/16O-ratio. After 10 h at 21.5 or 18.5 degrees C the delta18O-value increased by 0.4 or 0.3 per thousand per h, respectively, in samples (50 g) of chopped meat. The observed magnitude of changes might compensate for the geographical and seasonal differences. A precise origin assignment of the affected specimen on the base of delta18O-values of meat water is hence bound to be impossible.

  9. {sup 4}He fragments from the {sup 14}N + {sup 12}C collision at 35 MeV/nucleon and clustering in colliding nuclei

    SciTech Connect

    Takemoto, H.; Horiuchi, H.; Engel, A.; Ono, A.

    1996-07-01

    In order to study effects of clustering of colliding nuclei in the fragmentation process, the fragmentation of the {sup 14}N+{sup 12}C reaction at 35 MeV/nucleon is analyzed by antisymmetrized molecular dynamics. It is found that {sup 4}He fragments from {sup 12}C fragmentation are much more abundant than those from {sup 14}N fragmentation. Characters of {sup 4}He fragments from {sup 12}C fragmentation are investigated and it is found that this abundance in {sup 12}C fragmentation results from the three-alpha breakup in a short time scale where the excited states with excitation energy 7{endash}15 MeV play an important role. {copyright} {ital 1996 The American Physical Society.}

  10. Solving the Large Discrepancy Between Inclusive and Exclusive Measurements of the 8Li + 4He → 11B + n Reaction Cross Section at Astrophysical Energies

    NASA Astrophysics Data System (ADS)

    La Cognata, M.; Del Zoppo, A.; Alba, R.; Cherubini, S.; Colonna, N.; Di Pietro, A.; Figuera, P.; Gulino, M.; Lamia, L.; Musumarra, A.; Pellegriti, M. G.; Pizzone, R. G.; Rolfs, C.; Romano, S.; Spitaleri, C.; Tumino, A.

    2009-12-01

    A solution of the large discrepancy existing between inclusive and exclusive measurements of the 8Li + 4He → 11B + n reaction cross section at E cm < 3 MeV is evaluated. This problem has profound astrophysical relevance for this reaction is of great interest in big bang and r-process nucleosynthesis. By means of a novel technique, a comprehensive study of all existing 8Li + 4He → 11B + n cross section data is carried out, setting up a consistent picture in which all the inclusive measurements provide the reliable value of the cross section. New unambiguous signatures of the strong branch pattern non-uniformities, near the threshold of higher 11B excited levels, are presented and their possible origin, in terms of the cluster structure of the involved excited states of 11B and 12Bnuclei, is discussed.

  11. Systematic Vibration Studies on a Cryogen-Free ^3He/^4He Dilution Refrigerator for X-ray Spectroscopy at Storage Rings

    NASA Astrophysics Data System (ADS)

    Scholz, P. A.; Kraft-Bermuth, S.; Andrianov, V.

    2016-08-01

    High-precision X-ray spectroscopy of highly charged ions at storage rings provides a sensitive test of quantum electrodynamics in strong Coulomb fields. To increase the precision of such experiments, silicon microcalorimeters have already been applied successfully. To minimize the interruption of beam times due to maintenance, a new cryogen-free ^3He/^4He dilution refrigerator has been designed and is under commissioning. However, in cryogen-free systems microphonic noise due to vibrations contributes considerably to the overall noise and may limit the detector energy resolution. Therefore, we report on systematic vibration studies on a cryogen-free ^3He/^4He dilution refrigerator which is specially adapted for experiments at storage rings.

  12. Contraband detection using high-energy gamma rays from 16O*

    NASA Astrophysics Data System (ADS)

    Micklich, Bradley J.; Fink, Charles L.; Sagalovsky, Leonid; Smith, Donald L.

    1997-02-01

    High-energy monoenergetic gamma rays (6.13 and 7.12 MeV) from the decay of excited states of the 16O* nucleus are highly penetrating and thus offer potential for non- intrusive inspection of loaded containers for narcotics, explosives, and other contraband items. These excited states can be produced by irradiation of water with 14-MeV neutrons from a DT neutron generator or through the 19F(p,alpha)16O* reaction. Resonances in 19F(p,alpha)16O* at proton energies between 340 keV and 2 MeV allow use of a low-energy accelerator to provide a compact, portable gamma source of reasonable intensity. The present work provides estimates of gamma source parameters and suggests how various types of contraband could be detected. Gamma rays can be used to perform transmission or emission radiography of containers or other objects. Through the use of (gamma,n) and (gamma,fission) reactions, this technique is also capable of detecting special nuclear materials such as deuterium, lithium, beryllium, uranium, and plutonium. Analytic and Monte Carlo techniques are used to model empty and loaded container inspection for accelerator-produced gamma, radioisotope, and x-ray sources.

  13. A non-terrestrial 16O-rich isotopic composition for the protosolar nebula.

    PubMed

    Hashizume, Ko; Chaussidon, Marc

    2005-03-31

    The discovery in primitive components of meteorites of large oxygen isotopic variations that could not be attributed to mass-dependent fractionation effects has raised a fundamental question: what is the composition of the protosolar gas from which the host grains formed? This composition is probably preserved in the outer layers of the Sun, but the resolution of astronomical spectroscopic measurements is still too poor to be useful for comparison with planetary material. Here we report a precise determination of the oxygen isotopic composition of the solar wind from particles implanted in the outer hundreds of nanometres of metallic grains in the lunar regolith. These layers of the grains are enriched in 16O by >20 +/- 4 per thousand relative to the Earth, Mars and bulk meteorites, which implies the existence in the solar accretion disk of reactions--as yet unknown--that were able to change the 17O/16O and 18O/16O ratios in a way that was not dependent strictly on the mass of the isotope. Photochemical self-shielding of the CO gas irradiated by ultraviolet light may be one of these key processes, because it depends on the abundance of the isotopes, rather than their masses. PMID:15800617

  14. Contraband detection using high-energy gamma rays from {sup 16}O*

    SciTech Connect

    Micklich, B.J.; Fink, C.L.; Sagalovsky, L.; Smith, D.L.

    1996-12-01

    High-energy monoenergetic gamma rays (6.13 and 7.12 MeV) from the decay of excited states of the {sup 16}O* nucleus are highly penetrating and thus offer potential for non-intrusive inspection of loaded containers for narcotics, explosives, and other contraband items. These excited states can be produced by irradiation of water with 14-MeV neutrons from a DT neutron generator or through the {sup 19}F(p,{alpha}){sup 16}O* reaction. Resonances in {sup 19}F(p,{alpha}){sup 16}O* at proton energies between 340 keV and 2 MeV allow use of a low-energy accelerator to provide a compact, portable gamma source of reasonable intensity. The present work provides estimates of gamma source parameters and suggests how various types of contraband could be detected. Gamma rays can be used to perform transmission or emission radiography of containers or other objects. Through the use of ({gamma}, n) and ({gamma}, fission) reactions, this technique is also capable of detecting special nuclear materials such as deuterium, lithium, beryllium, uranium, and plutonium. Analytic and Monte Carlo techniques are used to model empty and loaded container inspection for accelerator-produced gamma, radioisotope, and x-ray sources.

  15. The ({sup 18}O, {sup 16}O) reaction as a probe for nuclear spectroscopy

    SciTech Connect

    Cappuzzello, F.; Bondì, M.; Nicolosi, D.; Tropea, S.; Agodi, A.; Carbone, D.; Cavallaro, M.; Cunsolo, A.; Borello-Lewin, T.; Rodrigues, M. R. D.; De Napoli, M.; Linares, R.

    2014-11-11

    The response of nuclei to the ({sup 18}O, {sup 16}O) two-neutron transfer reaction at 84 MeV incident energy has been systematically studied at the Catania INFN-LNS laboratory. The experiments were performed using several solid targets from light ({sup 9}Be, {sup 11}B, {sup 12,13}C, {sup 16}O, {sup 28}Si) to heavy ones ({sup 58,64}Ni, {sup 120}Sn, {sup 208}Pb). The {sup 16}O ejectiles were detected at forward angles by the MAGNEX magnetic spectrometer. Exploiting the large momentum acceptance (−10%, +14%) and solid angle (50 msr) of the spectrometer, energy spectra were obtained with a relevant yield up to about 20 MeV excitation energy. The application of the powerful trajectory reconstruction technique did allow to get energy spectra with energy resolution of about 150 keV and angular distributions with angular resolution better than 0.3°. A common feature observed with light nuclei is the appearance of unknown resonant structures at high excitation energy. The strong population of these latter together with the measured width can reveal the excitation of a collective mode connected with the transfer of a pair.

  16. 16O(n,α) cross section investigation using LENZ instrument at LANSCE

    NASA Astrophysics Data System (ADS)

    Lee, H. Y.; Mosby, S.; Haight, R. C.; White, M. C.

    2016-06-01

    Importance of studying the 16O(n,α) reaction is motivated by multiple nuclear applications. The Los Alamos Neutron Science Center (LANSCE) produces a white neutron spectrum ranging from thermal to several hundreds of MeV energies. We have recently developed the LENZ (Low Energy NZ-neutron induced charged particle detection) capability to measure high-precision (n,α) cross sections. In order to provide more reliable data, we have enhanced solid angle coverage, and improved signal-to-noise ratios and time-of-flight resolution by implementing digitizer waveform analysis. The LENZ was commissioned by studying the 59Co(n,α) reaction with neutron beams in early 2015. For the 16O(n,α) reaction, we investigate solid oxygen targets and make a relative measurement to a better known cross section, such as the 6Li(n,α) reaction in order to further reduce systematic uncertainty. We will discuss the progress of the 16O(n,α) study at LANSCE and the outlook for improving Hauser-Feshbah prediction on (n,p) reaction cross sections.

  17. Radiation-damage-controlled He diffusion and 4He/3He spectra in apatite: an example of mutually consistent results from the Grand Canyon (Invited)

    NASA Astrophysics Data System (ADS)

    Farley, K. A.; Flowers, R. M.

    2009-12-01

    Recent work indicates that He diffusion from apatite is impeded by the accumulation of radiation damage from actinide decay. Supporting evidence includes laboratory diffusion measurements as well as (U-Th)/He dates positively correlated with effective uranium (eU) concentration in certain geologic situations. Here we investigate whether the radiation damage effect can be identified in 4He concentration profiles, as it must be if the system behaves as we anticipate. Apatites from nearby igneous basement samples in the Upper Gorge of the Grand Canyon showing a strong date-eU correlation were proton irradiated, step-heated, and analyzed for 4He/3He spectra. The low eU apatites with younger He dates yielded nearly flat spectra, while the high eU apatites with older He dates yielded highly rounded spectra (see Figure). This implies that the higher eU apatites were partially retaining He while the lower eU apatites were still acting as an open system. Using the RDAAM kinetic model (Flowers et al. 2009) and local geologic constraints we confirm that this behavior is consistent with the observed differences in date and eU, providing compelling evidence that both the He dates and the 4He profiles are sensitive to radiation damage accumulation. Equally importantly, the combination of multiple samples with differing eU and thus differing 4He/3He spectra yields remarkably tight constraints on the time-temperature path experienced by these rocks, from ~90oC down to < 30oC.

  18. Background considerations for the 2H(7Be,3H)6Be experimental data II: Three-body continuum

    NASA Astrophysics Data System (ADS)

    Chae, K. Y.; Guimarães, V.

    2015-11-01

    The present article reports second background considerations for the experimentally obtained 2H(7Be,3H)6Be differential cross sections. The one-neutron transfer reaction was measured in inverse kinematics by using radioactive 7Be ( t 1/2 = 53.2 days) beams at the Holifield Radioactive Ion Beam Facility of the Oak Ridge National Laboratory in 2004 in order to search for the resonances in the unbound 6Be nucleus. Resonances in this nucleus would affect the 3He(3He,2 p)4He reaction rate of the proton-proton chain occurring in stars such as our sun. The result shows, however, that the direct transfer to 6Be resonances is not particularly strong compared to other reaction channels that can produce tritons in the exit channels. The goals of the present work is to better understand the cross section data from transfer reaction measurements by adopting background considerations using the three-body continuum.

  19. Chaos in the classical mechanics of bound and quasi-bound HX-4He complexes with X = F, Cl, Br, CN.

    PubMed

    Gamboa, Antonio; Hernández, Henar; Ramilowski, Jordan A; Losada, J C; Benito, R M; Borondo, F; Farrelly, David

    2009-10-01

    The classical dynamics of weakly bound floppy van der Waals complexes have been extensively studied in the past except for the weakest of all, i.e., those involving He atoms. These complexes are of considerable current interest in light of recent experimental work focussed on the study of molecules trapped in small droplets of the quantum solvent (4)He. Despite a number of quantum investigations, details on the dynamics of how quantum solvation occurs remain unclear. In this paper, the classical rotational dynamics of a series of van der Waals complexes, HX-(4)He with X = F, Cl, Br, CN, are studied. In all cases, the ground state dynamics are found to be almost entirely chaotic, in sharp contrast to other floppy complexes, such as HCl-Ar, for which chaos sets in only at relatively high energies. The consequences of this result for quantum solvation are discussed. We also investigate rotationally excited states with J = 1 which, except for HCN-(4)He, are actually resonances that decay by rotational pre-dissociation. PMID:19756276

  20. Cross sections and analyzing powers for (p,n) reactions on {sup 3}He and {sup 4}He at 346 MeV

    SciTech Connect

    Ihara, E.; Wakasa, T.; Dozono, M.; Imamura, T.; Kuroita, S.; Noro, T.; Sagara, K.; Sueta, T.; Tanabe, H.; Yamada, Y.; Hatanaka, K.; Kato, M.; Matsubara, H.; Okamura, H.; Tameshige, Y.; Tamii, A.; Sakemi, Y.; Sekiguchi, K.; Suda, K.

    2008-08-15

    The cross sections and analyzing powers for (p,n) reactions on {sup 3}He and {sup 4}He have been measured at a bombarding energy of T{sub p}=346 MeV and reaction angles of {theta}{sub lab}=9.4 deg. - 27 deg. The energy transfer spectra for {sup 3}He(p,n) at large {theta}{sub lab} ({>=}16 deg.) are dominated by quasielastic contributions and can be reasonably reproduced by plane-wave impulse approximation (PWIA) calculations for quasielastic scattering. By contrast, the known L=1 resonances in {sup 4}Li are clearly observed near the threshold in the {sup 4}He(p,n) spectra. Because these contributions are remarkable at small angles, the energy spectra are significantly different from those expected for quasielastic scattering. The data are compared with the PWIA calculations, and it is found that the quasielastic contributions are dominant at large {theta}{sub lab} ({>=}22 deg.). The nuclear correlation effects on the quasielastic peak for {sup 4}He(p,n) are also discussed.

  1. A Reestimate of the Protosolar (^2^H/^1^H)_p_ ratio from (^3^He/^4^He)_SW_ solar wind measurements.

    NASA Astrophysics Data System (ADS)

    Gautier, D.; Morel, P.

    1997-07-01

    We reanalyze the inference of the protosolar abundance of deuterium made by Geiss (1993, in Origin and Evolution of the Elements, Eds., N. Prantzos, E. Vangioni-Flam, M. Casse, Cambridge University Press, p. 90) from measurements of (^3^He/^4^He)_SW_ in the solar wind. We use an evolutionary solar model with microscopic diffusion, constrained to fit the present age, radius and luminosity, as well as the observed ratio of heavy elements to hydrogen. The protosolar (^2^H/^1^H)_p_ is obtained from the best fit of (^3^He/^4^He)_SW_. Taking for the protosolar (^3^He/^4^He)_p_ the value measured in Jupiter by the Galileo probe (Niemann et al., 1996Sci...272..846N), we derive (^2^H/^1^H)_p_=(3.01+/-0.17)x10^-5^. Compared to the present interstellar medium value (Linsky et al., 1993ApJ...402..694L), this result is compatible with models of the chemical evolution of the Galaxy in the solar neighborhood; it is also marginally compatible with the Jovian (^2^H/^1^H)_J_=(5+/-2)x10^-5^ ratio measured by Galileo.

  2. Cross-section measurement for the /sup 7/Li(n,n't)/sup 4/He reaction at 14. 74 MeV

    SciTech Connect

    Smith, D.L.; Meadows, J.W.; Bretscher, M.M.; Cox, S.A.

    1984-09-01

    The cross section for the /sup 7/Li(n,n't)/sup 4/He reaction is measured at an average neutron energy of 14.74 MeV, with a resolution of 0.324 MeV, relative to the /sup 238/U neutron-fission cross section. Tritium activities for the irradiated lithium-metal samples (enriched to 99.95% in /sup 7/Li) are deduced using a liquid-scintillation counting method which relies upon the tritiated-water standard from the US National Bureau of Standards. The measured cross section ratio of /sup 7/Li(n,n't)/sup 4/He to /sup 238/U neutron fission is 0.2523 (+- 2.2%). The derived /sup 7/Li(n,n't)/sup 4/He reaction cross section is 0.301 (+- 5.3%) barn, based on the ENDF/B-V value of 1.193 (+- 4.8%) barn for the /sup 238/U neutron-fission cross section. 59 references.

  3. Improving tritium determination from environmental water samples by the 3He ingrowth method by means of an ultrapure 4He spike

    NASA Astrophysics Data System (ADS)

    Major, Zoltan; Palcsu, Laszlo; Papp, Laszlo

    2010-05-01

    Clarke et al. (1976) described a new method based on mass spectrometric measurement of 3He to deter-mine low level tritium concentrations of water samples [1]. The method consists of three major steps: 1) The water samples are put into glass bulbs. The dissolved gases including helium are removed from the water by vacuum pumping. 2) The sample are stored for several months or years so that 3He atoms are produced from tritium decay. 3) The amount of the tritiogenic 3He is measured mass spectrometrically. Since then numeru-ous laboratories adopted this method [2-5] as noble gas mass spectrometers became commercially available. The measurements are usually calibrated by means of well known air aliquots, which in size can be compared to the helium amount from the tritium sample. The 3He/4He ratio of samples can differ considerably from that of air used for standardization. For this reason it has to be kept in mind that a possible discrimination of 3He by 4He is not necessarily corrected by the air stan-dards [3]. Additionally, the mass spectrometric sensi-tivities of the different helium isotopes depend on the pressure at the ion source [6]. In case of tritium meas-urements, the overall pressure of the helium in the mass spectrometer is much lower than that of the helium from the air calibration. We use air aliquots that contain 7•10-9 to 2•10-7 ccSTP of 4He and 5•10-15 to 1.5•10-13 ccSTP of 3He. The relative standard deviations of the calibration measurements vary between 1-2 %, and the non-linearity effect is always taken into account. The over-all helium amount in the mass spectrometer in case of a tritium sample is usually less than 3•10-10 ccSTP that derives, of cource, from the 4He [5]. As the amount of the calibration sample converges to that of tritium samples, we loose the good statistical error of the 3He measurement being counted by an electro-multiplier. It seems that the large diiference of the helium pressure in the ion source between a sample

  4. Realization of a 3He-4He Vapor-Pressure Thermometer for Temperatures Between 0.65 K and 5 K at LNE-CNAM

    NASA Astrophysics Data System (ADS)

    Sparasci, F.; Pitre, L.; Truong, D.; Risegari, L.; Hermier, Y.

    2011-01-01

    In the temperature range between 0.65 K and 5 K, the International Temperature Scale of 1990 (ITS-90) is based on 3He and 4He vapor-pressure thermometers. Between 0.65 K and 1 K, the ITS-90 overlaps with the Provisional Low Temperature Scale of 2000 (PLTS-2000), defined in term of the melting pressure of 3He. Some differences, up to more than 1 mK, exist between the two scales in the overlapping interval. The LNE-CNAM has recently started the construction of a 3He-4He vapor-pressure thermometer to realize the ITS-90 in its lowest subrange at the highest degree of accuracy. The device is provided with two separate vapor-pressure chambers, one for 3He and the other for 4He, built in a single copper block, and is installed in the experimental space of a dilution refrigerator. The vapor-pressure thermometer is designed to accommodate on the same copper block several transfer standards, an acoustic thermometer, and the 3He melting-pressure thermometer. This configuration is intended for realizing calibrations of transfer standards down to 0.65 K, for investigating the possibility to extend the acoustic thermometer below 4 K, and to perform a direct comparison between the ITS-90 and the PLTS-2000 in the overlapping temperature range, in order to study their differences. The realization of the system has been recently accomplished, and this report illustrates the characteristics of such an experimental device.

  5. Localization of [3H]nicotine, [3H]cytisine, [3H]epibatidine, and [125I]alpha-bungarotoxin binding sites in the brain of Macaca mulatta.

    PubMed

    Han, Zhi-Yan; Zoli, Michele; Cardona, Ana; Bourgeois, Jean-Pierre; Changeux, Jean-Pierre; Le Novère, Nicolas

    2003-06-16

    We determined the localization of [(3)H]nicotine, [(3)H]cytisine, [(3)H]epibatidine, and [(125)I]alpha-bungarotoxin binding sites in the brain of rhesus monkey by means of receptor autoradiography. The labelings by [(3)H]nicotine, [(3)H]cytisine, and [(3)H]epibatidine were highly concordant, except for epibatidine. Layer IV of some cortical areas, most thalamic nuclei, and presubiculum displayed high levels of labeling for the three ligands. Moderate levels of binding were detected in the subiculum, the septum, and the mesencephalon. Low levels were present in layers I-II and VI of the cortex, the cornu Ammonis, the dentate gyrus, and the amygdala. In addition, the level of epibatidine labeling was very high in the epithalamic nuclei and the interpeduncular nucleus, whereas labeling by nicotine and cytisine was very weak in the same regions. The distribution of [(125)I]alpha-bungarotoxin binding differed from the binding of the three agonists. The labeling was dense in layer I of most cortical areas, dentate gyrus, stratum lacunosum-moleculare of CA1 field, several thalamic nuclei, and medial habenula. A moderate labeling was found in layers V and VI of the prefrontal and frontal cortices, layer IV of primary visual cortex, amygdala, septum, hypothalamus, and some mesencenphalic nuclei. A weak signal was also detected in subiculum, claustrum, stratum oriens, and stratum lucidum of cornu Ammonis and also in some mesencephalic nuclei. The distribution of nicotine, cytisine, and epibatidine bindings corresponds broadly to the patterns observed in rodents, with the marked exception of the epithalamus. However, in monkey, those distributions match the distribution of alpha2 messenger RNA, rather than that of alpha4 transcripts as it exists in rodent brains. The distribution of the binding sites for alpha-bungarotoxin is larger in the brain of rhesus monkeys than in rodent brain, suggesting a more important role of alpha7 receptors in primates.

  6. Characteristics of [3H]sultopride binding to rat brain.

    PubMed

    Mizuchi, A; Kitagawa, N; Saruta, S; Miyachi, Y

    1982-10-15

    The binding of [3H]sultopride, a benzamide drug, to rat brain was investigated in vitro. Specific [3H]sultopride binding was observed in dopaminergic regions: striatum, nucleus accumbens, olfactory tubercle, substantia nigra, frontal cortex and anterior pituitary. Specific [3H]sultopride binding to striatum was saturable and had one high affinity binding site with a KD of 5.8 nM and a total density of receptors 25.7 pmol/g. [3H]Sultopride binding was stereoselectively displaced by (-)- and (+)-sultopride. Inhibition studies indicated that all neuroleptic drugs and dopamine were capable of displacing sultopride from its binding sites. A highly significant correlation was observed between IC50 values against [3H]sultopride and those against [3H]spiperone binding. Specific [3H]sultopride binding was highly dependent on the presence of sodium ions. The results suggest that the characteristics of sultopride binding sites seem to be similar to those of the D2-receptor labeled by spiperone and haloperidol. The sultopride binding site was highly dependent on the presence of sodium ions and may thus be characterized as a sodium-dependent D2-receptor.

  7. Fallout /sup 3/H ingestion in Akita, Japan

    SciTech Connect

    Hisamatsu, S.; Takizawa, Y.; Abe, T.; Katsumata, T.

    1987-09-01

    To study fallout /sup 3/H ingestion in Japan, 16 separate food group samples were collected from Akita during 1985. The /sup 3/H concentration in free water and that in a tissue-bound form were determined separately. The average /sup 3/H concentration in the tissue-bound form was 2.2 Bq L-1, 1.7 times higher than in the free water of the food. The ingestions of /sup 3/H in the tissue-bound form and as free water in the diet were 0.60 Bq d-1 and 1.0 Bq d-1, respectively. Cereals represented the food group that contributed the most to the ingestion of tissue-bound /sup 3/H. Total /sup 3/H ingestion was estimated to be 4.1 Bq d-1. The contribution of the tissue-bound form to the total ingestion was 15%, considerably lower than reported for Italian diets. The ratio of /sup 3/H ingestion in the tissue-bound form to the free water form in the diet was similar to the ratio reported for New York City.

  8. Characterization of [3H]palmitate- and [3H]ethanolamine-labelled proteins in the multicellular parasitic trematode Schistosoma mansoni.

    PubMed Central

    Wiest, P M; Tisdale, E J; Roberts, W L; Rosenberry, T L; Mahmoud, A A; Tartakoff, A M

    1988-01-01

    Biosynthetic labelling experiments with cercariae and schistosomula of the multicellular parasitic trematode Schistosoma mansoni were performed to determine whether [3H]palmitate or [3H]ethanolamine was incorporated into proteins. Parasites incorporated [3H]palmitate into numerous proteins, as judged by SDS/polyacrylamide-gel electrophoresis and fluorography. The radiolabel was resistant to extraction with chloroform, but sensitive to alkaline hydrolysis, indicating the presence of an ester bond. Further investigation of the major 22 kDa [3H]palmitate-labelled species showed that the label could be recovered in a Pronase fragment which bound detergent and had an apparent molecular mass of 1200 Da as determined by gel filtration on Sephadex LH-20. Schistosomula incubated with [3H]ethanolamine for up to 24 h incorporated this precursor into several proteins; labelled Pronase fragments recovered from the three most intensely labelled proteins were hydrophilic and had a molecular mass of approx. 200 Da. Furthermore, reductive methylation of such fragments showed that the [3H]ethanolamine bears a free amino group, indicating the lack of an amide linkage. We also evaluated the effect of phosphatidylinositol-specific phospholipase C from Staphylococcus aureus: [3H]palmitate-labelled proteins of schistosomula and surface-iodinated proteins were resistant to hydrolysis with this enzyme. In conclusion, [3H]palmitate and [3H]ethanolamine are incorporated into distinct proteins of cercariae and schistosomula which do not bear glycophospholipid anchors. The [3H]ethanolamine-labelled proteins represent a novel variety of protein modification. Images Fig. 1. Fig. 3. Fig. 5. PMID:3178767

  9. 2-D numerical simulations of groundwater flow, heat transfer and 4He transport — implications for the He terrestrial budget and the mantle helium heat imbalance

    NASA Astrophysics Data System (ADS)

    Castro, Maria Clara; Patriarche, Delphine; Goblet, Patrick

    2005-09-01

    Because helium and heat production results from a common source, a continental 4He crustal flux of 4.65 * 10 - 14 mol m - 2 s - 1 has been estimated based on heat flow considerations. In addition, because the observed mantle He / heat flux ratio at the proximity of mid-ocean ridges (6.6 * 10 - 14 mol J - 1 ) is significantly lower than the radiogenic production ratio (1.5 * 10 - 12 mol J - 1 ), the presence of a terrestrial helium-heat imbalance was suggested. The latter could be explained by the presence of a layered mantle in which removal of He is impeded from the lower mantle [R.K. O'Nions, E.R. Oxburgh, Heat and helium in the Earth, Nature 306 (1983) 429-431; E.R. Oxburgh, R.K. O'Nions, Helium loss, tectonics, and the terrestrial heat budget, Science 237 (1987) 1583-1588]. van Keken et al. [P.E. van Keken, C.J. Ballentine, D. Porcelli, A dynamical investigation of the heat and helium imbalance, Earth Planet, Sci. Lett. 188 (2001) 421-434] have recently claimed that the helium-heat imbalance remains a robust observation. Such conclusions, however, were reached under the assumption that a steady-state regime was in place for both tracers and that their transport properties are similar at least in the upper portion of the crust. Here, through 2-D simulations of groundwater flow, heat transfer and 4He transport carried out simultaneously in the Carrizo aquifer and surrounding formations in southwest Texas, we assess the legitimacy of earlier assumptions. Specifically, we show that the driving transport mechanisms for He and heat are of a fundamentally different nature for a high range of permeabilities ( k ≤ 10 - 16 m 2) found in metamorphic and volcanic rocks at all depths in the crust. The assumption that transport properties for these two tracers are similar in the crust is thus unsound. We also show that total 4He / heat flux ratios lower than radiogenic production ratios do not reflect a He deficit in the crust or mantle original reservoir. Instead, they

  10. Crossed-beam radical-radical reaction dynamics of O(3P)+C3H3-->H(2S)+C3H2O

    NASA Astrophysics Data System (ADS)

    Kwon, Lee-Kyoung; Nam, Mi-Ja; Youn, Sung-Eui; Joo, Sun-Kyu; Lee, Hohjai; Choi, Jong-Ho

    2006-05-01

    The radical-radical oxidation reaction, O(P3)+C3H3(propargyl)→H(S2)+C3H2O (propynal), was investigated using vacuum-ultraviolet laser-induced fluorescence spectroscopy in a crossed-beam configuration, together with ab initio and statistical calculations. The barrierless addition of O(P3) to C3H3 is calculated to form energy-rich addition complexes on the lowest doublet potential energy surface, which subsequently undergo direct decomposition steps leading to the major reaction products, H +C3H2O (propynal). According to the nascent H-atom Doppler-profile analysis, the average translational energy of the products and the fraction of the average transitional energy to the total available energy were determined to be 5.09±0.36kcal/mol and 0.077, respectively. On the basis of a comparison with statistical prior calculations, the reaction mechanism and the significant internal excitation of the polyatomic propynal product can be rationalized in terms of the formation of highly activated, short-lived addition-complex intermediates and the adiabaticity of the excess available energy along the reaction coordinate.

  11. An Observational Investigation of the Identity of B11244 (l-C3H+/C3H-)

    NASA Astrophysics Data System (ADS)

    McGuire, Brett A.; Carroll, P. Brandon; Gratier, Pierre; Guzmán, Viviana; Pety, Jerome; Roueff, Evelyne; Gerin, Maryvonne; Blake, Geoffrey A.; Remijan, Anthony J.

    2014-03-01

    Pety et al. have reported the detection of eight transitions of a closed-shell, linear molecule (B11244) in observations toward the Horsehead photodissociation region (PDR), which they attribute to the l-C3H+ cation. Recent high-level ab initio calculations have called this assignment into question; the anionic C3H- molecule has been suggested as a more likely candidate. Here, we examine observations of the Horsehead PDR, Sgr B2(N), TMC-1, and IRC+10216 in the context of both l-C3H+ and C3H-. We find no observational evidence of Ka = 1 lines, which should be present were the carrier indeed C3H-. Additionally, we find a strong anticorrelation between the presence of known molecular anions and B11244 in these regions. Finally, we discuss the formation and destruction chemistry of C3H- in the context of the physical conditions in the regions. Based on these results, we conclude there is little evidence to support the claim that the carrier is C3H-.

  12. (/sup 3/H) clonidine binding to rat hippocampal membranes

    SciTech Connect

    George, C.R.

    1982-02-01

    Alpha adrenergic receptor subtypes in rat hippocampal membranes were studied, using (/sup 3/H) clonidine as the radioactive ligand. On the basis of competitive binding studies, using the selective antagonist-prazosin, WB-4101, and yohimbine, (/sup 3/H) clonidine appeared to bind to a population of presynaptic sites that are pharmacologically similar to receptors previously classified as alpha 2. A computerized model that linearized and produced the best possible fit to the experimental data points indicated that (/sup 3/H) clonidine binds to a single population of receptors possessing equal affinity for the ligand. Binding data also indicated that rat hippo-campus contains significantly fewer (/sup 3/H)clonidine binding sites than rat cortex.

  13. Autoradiographic localization of (3H) gepirone in the rat brain

    SciTech Connect

    Bennett, J.E.; Matheson, G.K. )

    1990-02-26

    Gepirone is an anxiolytic compound active at the 5-HT{sub 1A} receptor site. The purpose of this study was to locate the ({sup 3}H)gepirone in the rat brain and to determine the quantity of gepirone in these locations. Male Sprague-Dawley rats were injected with (3H)gepirone (200 {mu}Ci/kg, i.v.) and decapitated 10 minutes later. To determine specific binding some animals were pretreated with cold gepirone (1 mg/kg) 15 minutes before the (3H)gepirone treatment. The brains were removed, frozen, sectioned, and fixed in formaldehyde vapors. Tritium sensitive film was exposed to the sections for 106 days. Using computerized imaging technology data were obtained from 104 brain sites. Overall, the quantity of (3H)gepirone in each site correlated proportionally with known 5-HT{sub 1A} (in vitro) receptor binding.

  14. Fallout sup 3 H in human tissue at Akita, Japan

    SciTech Connect

    Hisamatsu, S.; Takizawa, Y.; Itoh, M.; Ueno, K.; Katsumata, T.; Sakanoue, M. )

    1989-10-01

    The {sup 3}H concentration in Japanese human tissue samples is reported in this paper. Four brain, 10 liver, and nine lung samples from 11 cases were collected from Akita Prefecture in northern Japan from January to July 1986. The median of free-water {sup 3}H concentration was similar in these tissues and agreed well with the concentrations in the diet, including tap water. The median specific activity ratio of tissue-bound {sup 3}H to free-water {sup 3}H was 1.1 and was slightly lower than that in the diet. The specific activity ratio was also lower than that reported in the United States and significantly lower than in Italy.

  15. (/sup 3/H)-beta-endorphin binding in rat brain

    SciTech Connect

    Houghten, R.A.; Johnson, N.; Pasternak, G.W.

    1984-10-01

    The binding of (/sup 3/H)-beta-endorphin to rat brain homogenates is complex. Although Scatchard analysis of saturation studies yields a straight line, detailed competition studies are multiphasic, suggesting that even at low concentrations of the compound, the /sup 3/H-ligand is binding to more than one class of site. A portion of (/sup 3/H)-beta-endorphin binding is sensitive to low concentrations of morphine or D-Ala2-Leu5-enkephalin (less than 5 nM). The inhibition observed with each compound alone (5 nM) is the same as that seen with both together (each at 5 nM). Thus, the binding remaining in the presence of both morphine and the enkephalin does not correspond to either mu or delta sites. The portion of (/sup 3/H)-beta-endorphin binding that is inhibited under these conditions appears to be equally sensitive to both morphine and the enkephalin and may correspond to mu1 sites. Treating membrane homogenates with naloxonazine, a mu1 selective antagonist, lowers (/sup 3/H)-beta-endorphin binding to the same degree as morphine and D-Ala2-Leu5-enkephalin alone or together. This possible binding of (/sup 3/H)-beta-endorphin to mu1 sites is consistent with the role of mu1 sites in beta-endorphin analgesia and catalepsy in vivo.

  16. 16O excesses in olivine inclusions in Yamato-86009 and Murchison chondrites and their relation to CAIs.

    PubMed

    Hiyagon, H; Hashimoto, A

    1999-02-01

    In situ ion microprobe analyses of oxygen isotopes in Yamato-86009 and Murchison chondrites show that they contain abundant olivine-rich inclusions that have large oxygen-16 (16O) excesses, similar to those in spinel grains in calcium-aluminium-rich inclusions in Allende and other carbonaceous chondrites. The existence of 16O-enriched olivine-rich inclusions suggests that oxygen isotopic anomalies were more extensive in the early solar system than was previously thought and that their origin may be attributed to a nebular chemical process rather than to an unidentified 16O-rich carrier of presolar origin.

  17. Possible mechanisms of fragmentation of {sup 16}O nuclei with a momentum of 4.5 GeV/c per nucleon in track emulsions

    SciTech Connect

    Kotikov, E. A.

    2013-06-15

    The angular distributions of doubly charged fragments of {sup 16}O nuclei having a momentum of 4.5 GeV/c per nucleon and interacting with track-emulsion nuclei were studied. The experimental angular distributions of doubly charged fragments of a {sup 16}O nucleus are not described by the statistical model of the fragmentation of nuclei. The possible channels of fragmentation of {sup 16}O nuclei may include {sup 16}O {yields} 2{sup 8}Be {yields} 4{alpha}, {sup 16}O {yields} {sup 8}Be +{sup 8} Be* {yields} 4{alpha}, {sup 16}O {yields} 2{sup 8}Be* {yields} 4{alpha}, {sup 16}O {yields} {alpha}+{sup 12}C, {sup 16}O {yields} {alpha} +{sup 12}C* {yields} {alpha} + 3{alpha}, {sup 16}O {yields} {alpha} +{sup 12}C* {yields} {alpha} + p{alpha}{sup 7}Li, {sup 16}O {yields} {alpha} +{sup 12}C* {yields} {alpha} + 2{sup 6}Li, {sup 16}O {yields} {alpha} +{sup 12}C* {yields} {alpha} + pt2{alpha}, {sup 16}O {yields} Li + B, and {sup 16}O {yields} Li* + B*.

  18. Improved investigation of the 12C(α,γ)16O reaction

    NASA Astrophysics Data System (ADS)

    Kunz, R.; Hammer, J. W.; Jaeger, M.; Joos, K.-D.; Mayer, A.; Harissopulos, S.; Paradellis, Th.; Souliotis, G.; Staudt, G.

    2000-07-01

    The capture reaction 12C(α,γ)16O has been investigated in the energy range Ec.m.=0.96-2.6 MeV at the DYNAMITRON facility of the Institut für Strahlenphysik with an intense He+-beam of up to 480 μA. A setup of 3-4 HPGe detectors with active suppression on a turnable table has been used for the measurement of angular distributions, which is crucial to obtain information about E1 and E2 contributions.

  19. Covariance of Neutron Cross Sections for {sup 16}O through R-matrix Analysis

    SciTech Connect

    Kunieda, S.; Kawano, T.; Paris, M.; Hale, G.M.; Shibata, K.; Fukahori, T.

    2015-01-15

    Through the R-matrix analysis, neutron cross sections as well as the covariance are estimated for {sup 16}O in the resolved resonance range. Although we consider the current results are still preliminary, we present the summary of the cross section analysis and the results of data uncertainty/covariance, including those for the differential cross sections. It is found that the values obtained highlight consequences of nature in the theory as well as knowledge from measurements, which gives a realistic quantification of evaluated nuclear data covariances.

  20. Proton rapidity distributions from 60 GeV/n sup 16 O + Au collisions

    SciTech Connect

    Tonse, S.

    1990-05-01

    An analysis of the proton rapidity distribution in central {sup 16} O + Au collisions at 60 GeV/n measured in the NA35 streamer chamber detector at the CERN SPS is presented. The charge excess of positive particles over negative particles was measured. The rapidity distribution of the charge excess which can be associated with the primordial protons in the collision is studies in terms of the nuclear stopping power and is compared to the predictions of various models. 7 refs., 2 figs.

  1. Proton rapidity distributions from 60 GeV/n sup 16 O+Au collisions

    SciTech Connect

    Baechler, J.; Hoffman, M.; Runge, K.; Schmoetten, E. . Fakultaet fuer Physik); Bartke, J.; Gladysz, E. ); Bialkowska, H. ); Bock, R.; Brockmann, R.; Guerra, C.; Humanic, T.; Sandoval, A. ); Buncic, P.; Ljubicic, A.

    1990-05-01

    An analysis of the proton rapidity distribution in central {sup 16}O+Au collisions at 60 GeV/n measured in the NA35 streamer chamber detector at the CERN SPS is presented. The charge excess of positive particles over negative particles was measured. The rapidity distribution of the charge excess which can be associated with the primordial protons in the collision is studied in terms of the nuclear stopping power and is compared to the predictions of various models. 7 refs., 2 figs.

  2. Binding of [3H]palmitate to BSA.

    PubMed

    Elmadhoun, B M; Wang, G Q; Templeton, J F; Burczynski, F J

    1998-10-01

    Determination of the BSA-palmitate high-affinity binding constant (Ka) traditionally relied on the heptane-water partitioning technique. We used this technique to calculate Ka for the BSA-[3H]palmitate complex, to determine if Ka was independent of protein concentration, and to determine if the unbound [3H]palmitate concentration is constant at different BSA concentrations using constant BSA-to-palmitate molar ratios (range 1:1 to 1:4). After extensive extraction of non-[3H]palmitate radiolabeled substances, the heptane-to-buffer partition ratio, in the absence of BSA, was 702 +/- 19 (mean +/- SD, n = 6). This value was much lower than the predicted value of 1,376 and was highly dependent on which phase (organic or aqueous) initially contained the [3H]palmitic acid. The data were consistent with the notion of self-association of [3H]palmitate in the aqueous phase. Ka for the BSA-[3H]palmitate complex was determined to be similar (2.2 +/- 0.1) x 10(8) M-1 (mean +/- SD, P > 0.05) at all BSA concentrations studied. At each BSA-to-palmitate molar ratio, the equilibrium unbound ligand concentration was constant only at low BSA concentrations (<10 microM) and at low BSA-to-palmitate molar ratios (i.e., 1:1 and 1:2). At higher BSA concentrations and molar ratios, the unbound ligand concentration increased with an increase in protein concentration. Hepatocyte uptake using the manufacturer-supplied radiolabeled product was significantly higher than with the purified product, suggesting that a non-[3H]palmitate radiolabel is also a substrate for the uptake process.

  3. Asthenosphere–lithosphere interactions in Western Saudi Arabia: Inferences from 3He/4He in xenoliths and lava flows from Harrat Hutaymah

    USGS Publications Warehouse

    Konrad, Kevin;; Graham, David W; Thornber, Carl; Duncan, Robert A; Kent, Adam J.R.; Al-Amri, Abdulla

    2016-01-01

    Elevated 3He/4He in the western harrats has been observed only at Rahat (up to 11.8 RA; Murcia et al., 2013), a volcanic field situated above thinned lithosphere beneath the Makkah-Medinah-Nafud volcanic lineament. Previous work established that spinel lherzolites at Hutaymah are sourced near the lithosphere-asthenosphere boundary (LAB), while other xenolith types there are derived from shallower depths within the lithosphere itself (Thornber, 1992). Helium isotopes are consistent with melts originating near the LAB beneath many of the Arabian harrats, and any magma derived from the Afar mantle plume currently appears to be of minor importance.

  4. Experimental and theoretical study of the {sup 2}H(d-vector{gamma}){sup 4}He reaction below E{sub c.m.}=60 keV

    SciTech Connect

    Sabourov, K.; Ahmed, M.W.; Canon, S.R.; Crowley, B.; Joshi, K.; Kelley, J.H.; Nelson, S.O.; Perdue, B.A.; Schreiber, E.C.; Sabourov, A.; Tonchev, A.; Weller, H.R.; Wulf, E.A.; Prior, R.M.; Spraker, M.C.; Hofmann, H.M.; Trini, M.

    2004-12-01

    New measurements of the analyzing powers A{sub y} and T{sub 20} have been obtained for the {sup 2}H(d,{gamma}){sup 4}He reaction at a laboratory beam energy of 115 keV. A transition matrix element analysis results in a unique solution which indicates that the reaction proceeds by 55% E2, 29% E1, and 16% M2 radiation. These results are shown to be in good agreement with the results of a new refined resonating group model calculation. The impact of these results on the extrapolated value of the astrophysical S factor for this reaction is discussed.

  5. Simulation of 3He(d,p) 4He reaction and recent results of the experimental investigation of dp breakup reaction

    NASA Astrophysics Data System (ADS)

    Janek, M.; Kurilkin, P. K.; Tarjanyiova, G.; Ladygin, V. P.; Gurchin, Yu V.; Isupov, A. Yu; Karachuk, J.-T.; Khrenov, A. N.; Kurilkin, A. K.; Livanov, A. N.; Martinska, G.; Piyadin, S. M.; Reznikov, S. G.; Merts, S. P.; Batyuk, P. N.; Terekhin, A. A.; Vnukov, I. E.

    2016-02-01

    The feasibility study for the measurements of the polarization observables in the 3He(d,p) 4He reaction for DSS project using a part of the BM@N setup have been performed. Deuteron beam with energy of 1.5 GeV, magnet, 12 stations GEM tracker and TOF wall were used in simulations in order to obtain momentum resolution and to prove the separation of the secondary protons and deuterons. Summarized results of the dp breakup reactions with detection of two protons in coincidence for some kinematic configurations at energies from 300 to 500 MeV obtained in Nuclotron are presented.

  6. Excitation of the dynamical dipole in the charge asymmetric reaction 16O + 116Sn

    NASA Astrophysics Data System (ADS)

    Corsi, A.; Wieland, O.; Kravchuk, V. L.; Bracco, A.; Camera, F.; Benzoni, G.; Blasi, N.; Brambilla, S.; Crespi, F. C. L.; Giussani, A.; Leoni, S.; Million, B.; Montanari, D.; Moroni, A.; Gramegna, F.; Lanchais, A.; Mastinu, P.; Brekiesz, M.; Kmiecik, M.; Maj, A.; Bruno, M.; D'Agostino, M.; Geraci, E.; Vannini, G.; Barlini, S.; Casini, G.; Chiari, M.; Nannini, A.; Ordine, A.; Di Toro, M.; Rizzo, C.; Colonna, M.; Baran, V.

    2009-08-01

    The γ-ray emission from the dynamical dipole formed in heavy-ion collisions during the process leading to fusion was measured for the N/Z asymmetric reaction 16O + 116Sn at beam energies of 8.1 and 15.6 MeV/nucleon. High-energy γ-rays and charged particles were measured in coincidence with the heavy recoiling residual nuclei. The data are compared with those from the N/Z symmetric reaction 64Ni + 68Zn at bombarding energies of 4.7 and 7.8 MeV/nucleon, leading to the same CN with the same excitation energies as calculated from kinematics. The measured yield of the high-energy γ-rays from the 16O-induced reaction is found to exceed that of the thermalized CN and the excess yield increases with bombarding energy. The data are in rather good agreement with the predictions for the dynamical dipole emission based on the Boltzmann-Nordheim-Vlasov model. In addition, a comparison with existing data in the same mass region is performed to extract information on the dipole moment dependence.

  7. A study of the {sup 16}O (e, e'p) reaction at deep missing energies

    SciTech Connect

    Nilanga Liyanage

    1999-02-01

    The {sup 16}O(e,e'p) reaction was studied in the first physics experiment performed at Jefferson lab Hall A. In the quasielastic region cross sections were measured for both quasi parallel and perpendicular kinematics at q = 1000 MeV and {omega} = 445 MeV. From the data acquired in quasi parallel kinematics longitudinal and transverse response functions R{sub L} and R{sub T} were separated for E{sub miss} < 60 MeV. The perpendicular kinematics data were used to extract R{sub LT}, R{sub T}, and R{sub L } + V{sub TT}/V{sub L}R{sub TT} response functions for the same E{sub miss} range and for P{sub miss} < 310 MeV c. The {sub 16}O( e, e'p) cross section was measured in the dip region at q = 1026 MeV and {omega} = 586 MeV for 10 MeV < E{sub miss} < 320 MeV. This thesis presents the results for the missing energy continuum ( E{sub miss}>25 MeV) from this experiment.

  8. H2 16O line list for the study of atmospheres of Venus and Mars

    NASA Astrophysics Data System (ADS)

    Lavrentieva, N. N.; Voronin, B. A.; Fedorova, A. A.

    2015-01-01

    IR spectroscopy is an important method of remote measurement of H2 16O content in planetary atmospheres with initial spectroscopic information from the HITRAN, GEISA, etc., databases adapted for studies in the Earth's atmosphere. Unlike the Earth, the atmospheres of Mars and Venus mainly consist of carbon dioxide with a CO2 content of about 95%. In this paper, the line list of H2 16O is obtained on the basis of the BT2 line list (R.J. Barber, J. Tennyson, G.J. Harris, et al., Mon. Not. R. Astron. Soc. 368, 1087 (2006)). The BT2 line list containing information on the centers, intensities, and quantum identification of lines is supplemented with the line contour parameters: the self-broadening and carbon dioxide broadening coefficients and the temperature dependence coefficient at 296 K in the range of 0.001-30000 cm-1. Transitions with intensity values 10-30, 10-32, and 10-35 cm/molecule, the total number of which is 323310, 753529, and 2011072, respectively, were chosen from the BT2 line list.

  9. Reactivity impact of {sup 16}O thermal elastic-scattering nuclear data for some numerical and critical benchmark systems

    SciTech Connect

    Kozier, K. S.; Roubtsov, D.; Plompen, A. J. M.; Kopecky, S.

    2012-07-01

    The thermal neutron-elastic-scattering cross-section data for {sup 16}O used in various modern evaluated-nuclear-data libraries were reviewed and found to be generally too high compared with the best available experimental measurements. Some of the proposed revisions to the ENDF/B-VII.0 {sup 16}O data library and recent results from the TENDL system increase this discrepancy further. The reactivity impact of revising the {sup 16}O data downward to be consistent with the best measurements was tested using the JENDL-3.3 {sup 16}O cross-section values and was found to be very small in MCNP5 simulations of the UO{sub 2} and reactor-recycle MOX-fuel cases of the ANS Doppler-defect numerical benchmark. However, large reactivity differences of up to about 14 mk (1400 pcm) were observed using {sup 16}O data files from several evaluated-nuclear-data libraries in MCNP5 simulations of the Los Alamos National Laboratory HEU heavy-water solution thermal critical experiments, which were performed in the 1950's. The latter result suggests that new measurements using HEU in a heavy-water-moderated critical facility, such as the ZED-2 zero-power reactor at the Chalk River Laboratories, might help to resolve the discrepancy between the {sup 16}O thermal elastic-scattering cross-section values and thereby reduce or better define its uncertainty, although additional assessment work would be needed to confirm this. (authors)

  10. Measurement of the 2H(d ,p ) 3H reaction at astrophysical energies via the Trojan-horse method

    NASA Astrophysics Data System (ADS)

    Li, Chengbo; Wen, Qungang; Fu, Yuanyong; Zhou, Jing; Zhou, Shuhua; Meng, Qiuying; Spitaleri, C.; Tumino, A.; Pizzone, R. G.; Lamia, L.

    2015-08-01

    The study of the 2H(d ,p ) 3H reaction is very important for the nucleosynthesis in both the standard Big Bang and stellar evolution, as well as for the future fusion reactor's planning of energy production. The 2H(d ,p ) 3H bare nucleus astrophysical S (E ) factor has been measured indirectly at energies from about 400 keV down to several keV by means of the Trojan-horse method applied to the quasifree process 2H(6Li ,p t ) 4He induced at a lithium beam energy of 9.5 MeV, which is closer to the zero-quasifree-energy point. An accurate analysis leads to the determination of the Sbare(0 ) =56.7 ±2.0 keV b and of the corresponding electron screening potential Ue=13.2 ±4.3 eV. In addition, this work gives an updated test for the Trojan-horse nucleus invariance by comparing with previous indirect investigations using the 3He=(d +p ) breakup.

  11. Performance of compact liquid helium free 3He-4He dilution refrigerator directly coupled with GM cooler in TES microcalorimeter operation

    NASA Astrophysics Data System (ADS)

    Umeno, T.; Kamioka, Y.; Yoshida, S.; Maehata, K.; Ishibashi, K.; Takasaki, K.; Tanaka, K.

    2009-02-01

    A superconducting transition edge thermosensor (TES) microcalorimeter was cooled by a compact liquid-helium-free 3He-4He dilution refrigerator with loading a Gifford-McMahon (GM) cooler for detection of LX-ray photons emitted from an 241Am source. The first and second stages of the GM cooler are directly coupled with the first and the second precool heat exchangers of a stick shaped dilution unit through copper plates in the vacuum chamber, respectively. The circulating 3He-4He gas through the precooled heat exchangers is condensed into a liquid of condense mixture by the isoenthalpic expansion through the Joule-Thomson impedance. A cascade of two mixing chambers are employed for achieving sufficient cooling power. The helium-free dilution refrigerator performs the cooling power of 20 μW at 100 mK. The TES and SQUID chips suffered from mechanical vibrations induced by a reciprocating motion of the displacer of the GM cooler. Detection signals of LX-ray photons emitted from 241Am source were observed by operating the TES microcalorimeter in severe noise environment induced by mechanical vibrations.

  12. Comparison of the Effectiveness of Exposure to Low-LET Helium Particles ((4)He) and Gamma Rays ((137)Cs) on the Disruption of Cognitive Performance.

    PubMed

    Rabin, Bernard M; Carrihill-Knoll, Kirsty L; Shukitt-Hale, Barbara

    2015-09-01

    In this study, the effects of radiation exposure on cognitive performance were evaluated. Rats were exposed to either helium ((4)He) particles (1,000 MeV/n; 0.1-10 cGy; head only) or cesium (137)Cs gamma rays (50-400 cGy; whole body), after which their cognitive performance was evaluated. The results indicated that exposure to doses of (4)He particles as low as 0.1 cGy disrupted performance in a variety of cognitive tasks, including plus-maze performance (baseline anxiety), novel location recognition (spatial performance) and operant responding on an ascending fixed-ratio reinforcement schedule (motivation and responsiveness to changes in environmental contingencies) but not on novel object recognition performance (learning and memory). In contrast, after exposure to (137)Cs gamma rays only plus-maze performance was affected. There were no significant effects on any other task. Because exposure to both types of radiation produce oxidative stress, these results indicate that radiation-produced oxidative stress may be a necessary condition for the radiation-induced disruption of cognitive performance, but it is not a sufficient condition.

  13. Comparison of the Effectiveness of Exposure to Low-LET Helium Particles ((4)He) and Gamma Rays ((137)Cs) on the Disruption of Cognitive Performance.

    PubMed

    Rabin, Bernard M; Carrihill-Knoll, Kirsty L; Shukitt-Hale, Barbara

    2015-09-01

    In this study, the effects of radiation exposure on cognitive performance were evaluated. Rats were exposed to either helium ((4)He) particles (1,000 MeV/n; 0.1-10 cGy; head only) or cesium (137)Cs gamma rays (50-400 cGy; whole body), after which their cognitive performance was evaluated. The results indicated that exposure to doses of (4)He particles as low as 0.1 cGy disrupted performance in a variety of cognitive tasks, including plus-maze performance (baseline anxiety), novel location recognition (spatial performance) and operant responding on an ascending fixed-ratio reinforcement schedule (motivation and responsiveness to changes in environmental contingencies) but not on novel object recognition performance (learning and memory). In contrast, after exposure to (137)Cs gamma rays only plus-maze performance was affected. There were no significant effects on any other task. Because exposure to both types of radiation produce oxidative stress, these results indicate that radiation-produced oxidative stress may be a necessary condition for the radiation-induced disruption of cognitive performance, but it is not a sufficient condition. PMID:26284421

  14. Solar-flare implanted He-4/He-3 and solar-proton-produced Ne and Ar concentration profiles preserved in lunar rock 61016

    NASA Technical Reports Server (NTRS)

    Rao, M. N.; Garrison, D. H.; Bogard, D. D.; Reedy, R. C.

    1993-01-01

    Depth profiles for Ne-21, Ne-22, and Ar-38 isotopes from oriented lunar rock 61016 are reported. Concentration profiles of cosmogenic GCR+SCR (Galactic cosmic ray and solar cosmic ray-produced) isotopes are determined, quantitatively resolving neon and argon produced by energetic solar flares from that produced by Galactic cosmic rays. The SCR component is resolved from the GCR component as a function of shielding, and excellent agreement is found between experimental SCR production profiles for the isotopes and theoretically calculated values. A characteristic SW He-4/He-3 ratio of 3450 +/- 81, representing energies down to as few keV/amu. In slightly deeper samples an SRF He-4/He-3 ratio of 3450 +/- 725 is found for He particles with E larger than about 1 MeV/amu. These results indicate that the isotopic composition of SF He, averaged over the long term, is energy-dependent. An implanted Ne-20/Ne-22 ratio of 12.4 is measured in unetched samples, representing E greater than 1 MeV/amu, and a ratio of 11.6 is inferred in the samples, representing E larger than about 5 MeV/amu.

  15. Hydrochemistry and 18O/16O and 2H/1H Ratios of Ugandan Waters

    NASA Astrophysics Data System (ADS)

    Gebremichael, M. G.; Jasechko, S.

    2013-12-01

    Today, 70% of the 35 million people living in Uganda have access to an improved water source, ranking Uganda 148 out of 179 nations reporting in 2010 (Millennium Development Goals Indicators). 80% of Ugandans rely on groundwater as their primary drinking water source, collecting at springs or from shallow wells. Similarly, 80% of Ugandans rely upon agriculture - usually rain fed - as their primary income source. Despite lack of access to protected water sources faced by 10 million Ugandans, and the importance of the blue economy to Uganda's continued development, a country-wide investigation of the chemistry and the stable oxygen and hydrogen isotope compositions of waters has yet to be completed. Here we present 250 analyses of 18O/16O, 2H/1H and dissolved ion concentrations of Ugandan lakes, rivers, groundwaters and springs collected during July, 2013. We use the new data to characterize regional scale groundwater recharge sources, advection pathways and interactions with surface waters. Large lakes - Albert, Edward and Victoria - show increases in 18O/16O and 2H/1H ratios consistent with open water evaporation, and are shown to be distinct from nearby groundwaters, suggesting minimal recharge from large lakes to the subsurface. Salinities of eastern Ugandan groundwaters are elevated relative to samples collected from the central and western regions, suggesting that longer groundwater residence times and enhanced water-rock interactions characterize these waters. Springs from western Uganda show a shift in 18O/16O to higher values as a result of hydrothermal water-rock exchanges. Dissolved ion and noble gas concentrations show potential for use in assessing geothermal energy resources, perhaps aiding the Ugandan Ministry for Energy, Minerals and Development to meet their goal of increasing renewable energy from 4% (current) to 61% of total use by 2017 (Nyakabwa-Atwoki, 2013). Millennium Development Goals Indicators. mdgs.un.org/unsd/mdg/data.aspx Nyakabwa

  16. R-matrix description of particle energy spectra produced by low-energy 3H + 3H reactions

    DOE PAGES

    Brune, C. R.; Caggiano, J. A.; Sayre, D. B.; Bacher, A. D.; Hale, G. M.; Paris, M. W.

    2015-07-20

    An R-matrix model for three-body final states is presented and applied to a recent measurement of the neutron energy spectrum from the 3H + 3H→ 2n + α reaction. The calculation includes the n alpha and n n interactions in the final state, angular momentum conservation, antisymmetrization, and the interference between different channels. A good fit to the measured spectrum is obtained, where clear evidence for the 5He ground state is observed. The model is also used to predict the alpha-particle spectrum from 3H + 3H as well as particle spectra from 3He + 3He. The R-matrix approach presented heremore » is very general, and can be adapted to a wide variety of problems with three-body final states.« less

  17. (/sup 3/H)glucosamine and (/sup 3/H)proline radioautography of embryonic mouse dental basement membrane

    SciTech Connect

    Osman, M.; Ruch, J.V.

    1981-01-01

    (/sup 3/H)proline and (/sup 3/H)glucosamine radioautography was performed to analyze the labeling pattern of mouse embryonic dental basement membrane before and during odontoblast terminal differentiation. Sixteen- and eighteen-day-old first lower molars and trypsin-isolated enamel organs, as well as EDTA-isolated dental papillae, were used. Continuous labeling for 12 to 24 hr was required with (/sup 3/H)proline to obtain a clear labeling of epithelial-mesenchymal junction in intact tooth germs or accumulation of surface label in trypsin-isolated enamel organs. With (/sup 3/H)glucosamine, after 6-hr labeling, the epithelial-mesenchymal junction was heavily labeled and the trypsin-isolated enamel organs accumulated substantial amounts of surface label, corresponding to the redeposited basement membrane. At Day 16 stage, these labels always had a uniform distribution and decreased during chase without any redistribution. At Day 18 stage, when the terminal differentiation of odontoblasts occurred the label accumulated in a unique pattern: much more label was at the epithelial surface corresponding to the top of the cusps than in the apical parts. During chase and only in intact tooth germs epithelial surfaces which had labeled poorly during pulse became labeled, but those labeling heavily during pulse lost label. This pattern existed only in the presence of mesenchyme. EDTA treatment of (/sup 3/H)glucosamine-labeled teeth enabled us to obtain isolated dental papillae with surface label. Distribution of this label was exactly the same as that for the epithelial-mesenchymal junction of intact teeth. During chase, these dental papillae completely lost the surface label. The mesenchyme seen to control the synthesis and/or the degradation of epithelially derived (/sup 3/H)glucosamine-labeled material.

  18. Phenomenological and semi-microscopic analysis for 16O and 12C elastically scattering on the nucleus of 16O and 12C at Energies near the Coulomb barrier

    NASA Astrophysics Data System (ADS)

    Hamada, Sh; Burtebayev, N.; Amangeldi, N.; Gridnev, K. A.; Rusek, K.; Kerimkulov, Zh; Maltsev, N.

    2012-09-01

    The nuclear burning process proceeds from the conservation of the most abundant element hydrogen to helium, then from helium to carbon and oxygen, and then from these to heavier elements. Some of the key reactions for the carbon and oxygen burning stages of the nucleosynthesis are 12C+12C and 16O+16O leading to all possible final states. This paper contains the experimental measurements of 12C+12C and 16O+16O angular distributions performed at the cyclotron DC-60 in Astana, Kazakhstan. The extracted beam of 16O and 12C was accelerated up to two energies 1.75 and 1.5 MeV/n and then directed to an Al2O3 target of thickness 20 μg/cm2 and a carbon self-supporting target of thickness 17.4 μg/cm2. The angular distribution calculations were performed using both the phenomenological optical potential (SPI-GENOA) code and the double folding potential (FRESCO) code.

  19. Enhancing the branching ratios in the dissociation channels for O{sup 16}O{sup 16}O{sup 18} molecule by designing optimum laser pulses: A study using stochastic optimization

    SciTech Connect

    Talukder, Srijeeta; Chaudhury, Pinaki; Sen, Shrabani; Sharma, Rahul; Adhikari, Satrajit

    2015-10-14

    We propose a strategy of using a stochastic optimization technique, namely, simulated annealing to design optimum laser pulses (both IR and UV) to achieve greater fluxes along the two dissociating channels (O{sup 18} + O{sup 16}O{sup 16} and O{sup 16} + O{sup 16}O{sup 18}) in O{sup 16}O{sup 16}O{sup 18} molecule. We show that the integrated fluxes obtained along the targeted dissociating channel is larger with the optimized pulse than with the unoptimized one. The flux ratios are also more impressive with the optimized pulse than with the unoptimized one. We also look at the evolution contours of the wavefunctions along the two channels with time after the actions of both the IR and UV pulses and compare the profiles for unoptimized (initial) and optimized fields for better understanding the results that we achieve. We also report the pulse parameters obtained as well as the final shapes they take.

  20. Specific [(3)H]tryptophan binding sites in rat brain.

    PubMed

    Wong, P T; Lee, H S; Tan, C H; Teo, W L

    1989-01-01

    [(3)H]Tryptophan binds to a single population of sites in the rat cortical synaptosomal membranes. The binding is reversible and follows the law of mass action. By saturation studies using increasing concentration of [(3)H]tryptophan with decreasing specific radioactivity, the apparent K(d) obtained was approx. 0.8 ?M and the B(max) 110 pmol/mg protein. However, the IC(50) obtained for unlabelled tryptophan in displacing [(3)H]tryptophan binding (3.5 nM) was 0.26 ?M. All six naturally occurring aromatic amino acids studied displaced [(3)H]tryptophan binding with tryptophan and phenylalanine showing higher apparent affinity than histidine, tyrosine, dihydroxyphenylalanine and 5-hydroxytryptophan. These binding sites are proteins in nature as they are sensitive to trypsin and ?-chymotrypsin. It is observed that about 37% of the sites seem to be protected from the proteolytic enzymes by the membrane structure. Furthermore, they are extremely sensitive to phospholipase A(2) presumably because altered membrane phospholipids conduce a conformational change in the binding protein. A considerable degree of stereospecificity was demonstrated with the affinity for l-tryptophan about 90 times higher than that for d-tryptophan. The affinity for l-phenylalanine was 8 times higher than that for d-phenylalanine. Ligand specificity for the aromatic amino acids is remarkable as hydrocinnamic acid, 2-phenylethylamine, 5-hydroxytryptamine, histamine, dopamine, ?-aminobutyric acid, glutamic acid and taurine did not displace [(3)H]tryptophan binding. Therefore, these sites are termed aromatic amino acid binding sites (AABS). Whether or not AABS are involved in neuromodulation at the synapse awaits clarification. If so, the endogenous ligand for the AABS may well be tryptophan.

  1. Kinetics of the reaction of the heaviest hydrogen atom with H2, the 4Heμ + H2 → 4HeμH + H reaction: experiments, accurate quantal calculations, and variational transition state theory, including kinetic isotope effects for a factor of 36.1 in isotopic mass.

    PubMed

    Fleming, Donald G; Arseneau, Donald J; Sukhorukov, Oleksandr; Brewer, Jess H; Mielke, Steven L; Truhlar, Donald G; Schatz, George C; Garrett, Bruce C; Peterson, Kirk A

    2011-11-14

    The neutral muonic helium atom (4)Heμ, in which one of the electrons of He is replaced by a negative muon, may be effectively regarded as the heaviest isotope of the hydrogen atom, with a mass of 4.115 amu. We report details of the first muon spin rotation (μSR) measurements of the chemical reaction rate constant of (4)Heμ with molecular hydrogen, (4)Heμ + H(2) → (4)HeμH + H, at temperatures of 295.5, 405, and 500 K, as well as a μSR measurement of the hyperfine coupling constant of muonic He at high pressures. The experimental rate constants, k(Heμ), are compared with the predictions of accurate quantum mechanical (QM) dynamics calculations carried out on a well converged Born-Huang (BH) potential energy surface, based on complete configuration interaction calculations and including a Born-Oppenheimer diagonal correction. At the two highest measured temperatures the agreement between the quantum theory and experiment is good to excellent, well within experimental uncertainties that include an estimate of possible systematic error, but at 295.5 K the quantum calculations for k(Heμ) are below the experimental value by 2.1 times the experimental uncertainty estimates. Possible reasons for this discrepancy are discussed. Variational transition state theory calculations with multidimensional tunneling have also been carried out for k(Heμ) on the BH surface, and they agree with the accurate QM rate constants to within 30% over a wider temperature range of 200-1000 K. Comparisons between theory and experiment are also presented for the rate constants for both the D + H(2) and Mu + H(2) reactions in a novel study of kinetic isotope effects for the H + H(2) reactions over a factor of 36.1 in isotopic mass of the atomic reactant.

  2. 12C\\(α,γ\\)16O: The Key Reaction in Stellar Nucleosynthesis

    NASA Astrophysics Data System (ADS)

    Kunz, R.; Jaeger, M.; Mayer, A.; Hammer, J. W.; Staudt, G.; Harissopulos, S.; Paradellis, T.

    2001-04-01

    The angular distributions of γ rays from the 12C\\(α,γ\\)16O reaction have been measured at 20 energy points in the energy range Ecm = 0.95 to 2.8 MeV. The sensitivity of the present experiment compared to previous direct investigations was raised by 1-2 orders of magnitude, by using an array of highly efficient ( 100%) Ge detectors shielded actively with BGOs, as well as high beam currents of up to 500 μA that were provided by the Stuttgart Dynamitron accelerator. The SE1 and SE2 factors deduced from the γ angular distributions have been extrapolated to the range of helium burning temperatures applying the R-matrix method, which yielded S300E1 = \\(76+/-20\\) keV b and S300E2 = \\(85+/-30\\) keV b.

  3. 12C(alpha,gamma)16O: the key reaction in stellar nucleosynthesis.

    PubMed

    Kunz, R; Jaeger, M; Mayer, A; Hammer, J W; Staudt, G; Harissopulos, S; Paradellis, T

    2001-04-01

    The angular distributions of gamma rays from the 12C(alpha,gamma)16O reaction have been measured at 20 energy points in the energy range E(cm) = 0.95 to 2.8 MeV. The sensitivity of the present experiment compared to previous direct investigations was raised by 1-2 orders of magnitude, by using an array of highly efficient ( 100%) Ge detectors shielded actively with BGOs, as well as high beam currents of up to 500 microA that were provided by the Stuttgart Dynamitron accelerator. The S(E1) and S(E2) factors deduced from the gamma angular distributions have been extrapolated to the range of helium burning temperatures applying the R-matrix method, which yielded S(300)(E1) = (76+/-20) keV b and S(300)(E2) = (85+/-30) keV b.

  4. Elastic scattering of polarised deuterons from 16O at 200, 400 and 700 MeV

    NASA Astrophysics Data System (ADS)

    van Sen, Nguyen; Yanlin, Ye; Arvieux, J.; Gaillard, G.; Bonin, B.; Boudard, A.; Bruge, G.; Lugol, J. C.; Hasegawa, T.; Soga, F.; Antonuk, L. E.; Cameron, J. M.; Lam, S. T.; Neilson, G. C.; Roy, G.; Sheppard, D. M.; Babinet, R.

    1987-03-01

    Angular distributions of cross section, and Ay and Ayy analysing powers were measured for polarised deuteron elastic scattering from 16O at 200, 400 and 700 MeV. The data at 200 MeV bear evidence of the nuclear rainbow phenomenon while those at 400 and 700 MeV are reminiscent of the proton scattering results at equivalent energies. The data were analysed in terms of the optical model. The real central potential shape changes from an attractive Woods-Saxon form at 200 MeV to a wine-bottle-bottom form with a repulsive interior at 700 MeV. The total reaction cross sections deduced display a clear nuclear transparency effect in the present energy domain in agreement with predictions from the Glauber theory optical limit. Comparison with previous results for 40Ca and 58Ni targets is made.

  5. Development of {gamma}-ray detectors for {sup 16}O(p,p'{gamma}) experiment

    SciTech Connect

    Mori, T.; Izumi, T.; Ou, I.; Yano, T.; Sakuda, M.; Tamii, A.; Suzuki, T.; Yosoi, M.

    2012-11-12

    The {gamma} ray production in neutral-current (NC) neutrino-oxygen interaction is very important to the detection of neutrinos from supernova explosion in a neutrino experiment, since those {gamma} rays can become extra signals or unexpected background in the energy region from 5 MeV to 30 MeV. We propose the experiment to measure {gamma} rays in {sup 16}O(p,p') reaction at Research Center for Nuclear Physics (RCNP, Osaka) to provide good information on the {gamma}-ray emission spectra in neutrino-oxygen reactions. We present the design of {gamma}-ray detectors (NaI, CsI, HPGe), which will be used in proposed experiment.

  6. Evidence of complete fusion in the subbarrier {sup 16}O+{sup 238}U reaction

    SciTech Connect

    Nishio, K. Ikezoe, H.; Asai, M.; Tsukada, K.; Mitsuoka, S.; Tsuruta, K.; Satou, K.; Lin, C. J.; Ohsawa, T.

    2006-08-15

    Evaporation residue cross sections in the {sup 16}O+{sup 238}U reaction were measured for the energy range from above-to extreme subbarrier. We used a He-gas-jet system to transport the fusion products, and the {alpha} decay of the evaporation residues was measured by using a rotating wheel system. The measured cross sections for {sup 248,249,250}Fm are reproduced by a statistical model calculation, for which partial cross sections are calculated by a coupled-channel model taking into account the prolate deformation of {sup 238}U. We conclude that complete fusion is the main process in the subbarrier energy region, and quasifission is not an important channel.

  7. A New Decay Path in the {sup 12}C+{sup 16}O Radiative Capture Reaction

    SciTech Connect

    Courtin, S.; Lebhertz, D.; Haas, F.; Beck, C.; Michalon, A.; Salsac, M.-D.; Jenkins, D. G.; Marley, P.; Lister, C. J.

    2009-03-04

    The {sup 12}C({sup 16}O,{gamma}){sup 28}Si radiative capture reaction has been studied at energies close to the Coulomb barrier at Triumf (Vancouver) using the Dragon spectrometer and its associated BGO array. It has been observed that the {gamma} decay flux proceeds mainly via states around 10-11 MeV and via the direct feeding of the {sup 28}Si 3{sub 1}{sup -}(6879 keV) and 4{sub 2}{sup +}(6888 keV) deformed states. A discussion is presented about this selective feeding as well as perspectives for the use of novel detection systems for the study of light heavy-ion radiative capture reactions.

  8. Five-body calculation with Pauli constraint for shell- and cluster-structure in 16O

    NASA Astrophysics Data System (ADS)

    Horiuchi, Wataru; Suzuki, Yasuyuki

    2016-07-01

    A 12C+four-nucleon (4N) five-body model is applied for the ground and first excited states of 16O. The 4N configurations are selected in a wide Hilbert space under the fulfillment of the Pauli principle excluding the occupied orbits in 12C. The energies of both the states are obtained in excellent agreement with experiment. Analysis of the wave functions indicates a spatially localized alpha-particle-like cluster structure for the excited state and a shell-model-like delocalized structure for the ground state. The difficulty of describing the cluster structure by a standard shell model approach is discussed by calculating components of the harmonic-oscillator quanta in the wave functions.

  9. Helium and neon isotopes in phenocrysts from Samoan lavas: Evidence for heterogeneity in the terrestrial high 3He/ 4He mantle

    NASA Astrophysics Data System (ADS)

    Jackson, Matthew G.; Kurz, Mark D.; Hart, Stanley R.

    2009-10-01

    We report the first neon isotope measurements on phenocrysts from subaerial and submarine Samoan lavas. These new data complement existing Ne-isotope data from Samoan peridotite xenoliths (Poreda, R.J., Farley, K.A.,1992. Rare gases in Samoan xenoliths. Earth Planet. Sci. Lett. 113, 689 129-144). Neon isotopes were measured in magmatic phenocrysts separated from nine shield-stage lavas from 5 Samoan volcanoes, including Ofu, Ta'u, Vailulu'u, Malumalu and Savai'i. Phenocrysts from subaerial Samoan lavas have higher 20Ne/ 22Ne than submarine phenocrysts, which may suggest different atmospheric contamination mechanisms for these two different eruptive environments. Olivine phenocrysts from a subaerial Ta'u lava exhibit the highest 20Ne/ 22Ne (11.33±0.08, 1σ) value in this study. Two subaerial Samoan samples from Ofu Island with high 3He/ 4He ratios (Ofu-04-06 and Ofu-04-03; 34 and 24 Ra [ratio to atmosphere], respectively) also have elevated 20Ne/ 22Ne ratios relative to air, and in a three-isotope neon plot the Ofu samples are indistinguishable from measurements made on high 3He/ 4He lavas from Hawaii, Iceland and Galapagos. The similarity of helium and neon isotopes in Ofu and Hawaii-Iceland-Galapagos is remarkable given the distinctions in 87Sr/ 86Sr (0.70458 for Ofu vs. 0.70329-0.70368 for Hawaii-Iceland-Galapagos) and 143Nd/ 144Nd (Ofu's 0.51283 vs. 0.51294-0.51297 for Hawaii-Iceland-Galapagos) in high 3He/ 4He lavas from these localities. Thus, the occurrence of similar helium and neon isotope compositions in lavas from these 4 hotspots does not appear to be linked to their variable Sr and Nd isotope compositions, and demonstrates a complex relationship between the isotopes of noble gases and the more refractory radiogenic isotopes. Additionally, we observe strongly nucleogenic neon isotopes in one the most isotopically-enriched ( 87Sr/ 86Sr > 0.718) Samoan lavas. This observation is consistent with the presence of recycled, continentally-derived marine

  10. Deformation effects on sub-barrier fusion cross sections in 16O+174,176Yb

    NASA Astrophysics Data System (ADS)

    Rajbongshi, Tapan; Kalita, K.; Nath, S.; Gehlot, J.; Banerjee, Tathagata; Mukul, Ish; Dubey, R.; Madhavan, N.; Lin, C. J.; Shamlath, A.; Laveen, P. V.; Shareef, M.; Kumar, Neeraj; Jisha, P.; Sharma, P.

    2016-05-01

    Background: Couplings with various reaction channels are known to enhance sub-barrier fusion cross sections by several orders in magnitude. However, a few open questions still remain. For example, the influence of higher order static deformations on sub-barrier fusion cross sections is yet to be comprehensively understood. Purpose: We study the role of hexadecapole nuclear deformation effect on sub-barrier fusion cross sections. Also, this work aims to extract hexadecapole deformation (β4) in nuclei in the lanthanide region. Method: The evaporation residue (ER) excitation functions for 16O+174,176Yb were measured at laboratory beam energies (Elab) in the range of 64.6-103.6 MeV. Measurements were carried out by employing the recoil mass spectrometer Heavy Ion Reaction Analyzer (HIRA) at IUAC, New Delhi. Fusion barrier distributions (BDs) were extracted from data. Results from the experiment were subjected to coupled-channels analysis, in which β4 was varied as a free parameter. Results: Experimental fusion cross sections at energies below the barrier expectedly showed strong enhancement compared to the predictions from the one-dimensional barrier penetration model. Data were satisfactorily reproduced after inclusion of negative β4 for both the targets in the coupled-channels calculation. Conclusions: The significant role of hexadecapole deformation was observed in the sub-barrier fusion of 16O+174,176Yb. The proposed value of β4 reproduced the measured fusion excitation function reasonably well. The BDs from these data were also extracted but no definitive conclusions could be drawn from them.

  11. The 3 A Band System in the Spectrum of the 13C 16O Molecule

    NASA Astrophysics Data System (ADS)

    Hakalla, R.; Kępa, R.; Rytel, M.; Zachwieja, M.

    1999-10-01

    In the emission spectrum of the carbon monoxide 13C16O isotopic molecule three bands comprising about 1820 lines of the 3A band system (c3Π-a3Π) were recorded and analyzed. The 0-0 and 0-1 bands of this system were photographed for the first time and the 0-2 band was rephotographed by using methods of conventional high-resolution spectroscopy. The result of the rotational band analysis includes expanding of the spectrum interpretation up to J = 25 as well as the identification of four previously unobserved branches P13, R13, P31, and R31. Because of strong perturbations in the c3Π (v = 0) state, the calculation of the rovibronic structure constants was performed only for the lower a3Π state. By using a calculation based on a nonlinear least-squares method, an effective Hamiltonian of Brown [J. M. Brown, E. A. Colbourn, J. K. G. Watson, and F. D. Wayne, J. Mol. Spectrosc. 74, 294-318 (1979)] and a separative procedure proposed by Curl-Dane-Watson [R. F. Curl and C. B. Dane, J. Mol. Spectrosc. 128, 406-412 (1988); J. K. G. Watson, J. Mol. Spectrosc. 138, 302-308 (1989)], it was possible to derive the rotational structure constants for the v = 0, 1, and 2 levels for the a3Π state in the 13C16O isotopic molecule. Term values for the c3Π (v = 0) level and the equilibrium molecular constants for the a3Π state also are reported.

  12. The 3A Band System in the Spectrum of the (13)C(16)O Molecule.

    PubMed

    Hakalla; Kepa; Rytel; Zachwieja

    1999-10-01

    In the emission spectrum of the carbon monoxide (13)C(16)O isotopic molecule three bands comprising about 1820 lines of the 3A band system (c(3)Pi-a(3)Pi) were recorded and analyzed. The 0-0 and 0-1 bands of this system were photographed for the first time and the 0-2 band was rephotographed by using methods of conventional high-resolution spectroscopy. The result of the rotational band analysis includes expanding of the spectrum interpretation up to J = 25 as well as the identification of four previously unobserved branches P(13), R(13), P(31), and R(31). Because of strong perturbations in the c(3)Pi (v = 0) state, the calculation of the rovibronic structure constants was performed only for the lower a(3)Pi state. By using a calculation based on a nonlinear least-squares method, an effective Hamiltonian of Brown [J. M. Brown, E. A. Colbourn, J. K. G. Watson, and F. D. Wayne, J. Mol. Spectrosc. 74, 294-318 (1979)] and a separative procedure proposed by Curl-Dane-Watson [R. F. Curl and C. B. Dane, J. Mol. Spectrosc. 128, 406-412 (1988); J. K. G. Watson, J. Mol. Spectrosc. 138, 302-308 (1989)], it was possible to derive the rotational structure constants for the v = 0, 1, and 2 levels for the a(3)Pi state in the (13)C(16)O isotopic molecule. Term values for the c(3)Pi (v = 0) level and the equilibrium molecular constants for the a(3)Pi state also are reported. Copyright 1999 Academic Press.

  13. Robust MS quantification method for phospho-peptides using 18O/16O labeling

    PubMed Central

    Andersen, Claus A; Gotta, Stefano; Magnoni, Letizia; Raggiaschi, Roberto; Kremer, Andreas; Terstappen, Georg C

    2009-01-01

    Background Quantitative measurements of specific protein phosphorylation sites, as presented here, can be used to investigate signal transduction pathways, which is an important aspect of cell dynamics. The presented method quantitatively compares peptide abundances from experiments using 18O/16O labeling starting from elaborated MS spectra. It was originally developed to study signaling cascades activated by amyloid-β treatment of neurons used as a cellular model system with relevance to Alzheimer's disease, but is generally applicable. Results The presented method assesses, in complete cell lysates, the degree of phosphorylation of specific peptide residues from MS spectra using 18O/16O labeling. The abundance of each observed phospho-peptide from two cell states was estimated from three overlapping isotope contours. The influence of peptide-specific labeling efficiency was removed by performing a label swapped experiment and assuming that the labeling efficiency was unchanged upon label swapping. Different degrees of phosphorylation were reported using the fold change measure which was extended with a confidence interval found to reflect the quality of the underlying spectra. Furthermore a new way of method assessment using simulated data is presented. Using simulated data generated in a manner mimicking real data it was possible to show the method's robustness both with increasing noise levels and with decreasing labeling efficiency. Conclusion The fold change error assessable on simulated data was on average 0.16 (median 0.10) with an error-to-signal ratio and labeling efficiency distributions similar to the ones found in the experimentally observed spectra. Applied to experimentally observed spectra a very good match was found to the model (<10% error for 85% of spectra) with a high degree of robustness, as assessed by data removal. This new method can thus be used for quantitative signal cascade analysis of total cell extracts in a high throughput mode

  14. Arabidopsis C3H14 and C3H15 have overlapping roles in the regulation of secondary wall thickening and anther development.

    PubMed

    Chai, Guohua; Kong, Yingzhen; Zhu, Ming; Yu, Li; Qi, Guang; Tang, Xianfeng; Wang, Zengguang; Cao, Yingping; Yu, Changjiang; Zhou, Gongke

    2015-05-01

    Plant tandem CCCH zinc finger (TZF) proteins play diverse roles in developmental and adaptive processes. Arabidopsis C3H14 has been shown to act as a potential regulator of secondary wall biosynthesis. However, there is lack of direct evidence to support its functions in Arabidopsis. It is demonstrated here that C3H14 and its homologue C3H15 redundantly regulate secondary wall formation and that they additionally function in anther development. Plants with double, but not single, T-DNA mutants for C3H14 or C3H15 have few pollen grains and thinner stem secondary walls than the wild type. Plants homozygous for c3h14 and heterozygous for c3h15 [c3h14 c3h15(±)] have slightly thinner secondary walls than plants heterozygous for c3h14 and homozygous for c3h15 [c3h14(±) c3h15], and c3h14(±) c3h15 have lower fertility. Overexpression of C3H14 or C3H15 led to increased secondary wall thickness in stems and the ectopic deposition of secondary walls in various tissues, but did not affect anther morphology. Transcript profiles from the C3H14/15 overexpression and c3h14 c3h15 plants revealed marked changes in the expression of many genes associated with cell wall metabolism and pollen formation. Subcellular localization and biochemical analyses suggest that C3H14/15 might function at both the transcriptional and post-transcriptional levels.

  15. Determination of the {sup 22}Ne{sub nucl}/{sup 4}He{sub rad} ratio in natural uranium-rich fluorite by mass spectrometry

    SciTech Connect

    Sole, Jesus; Pi, Teresa

    2006-10-15

    A determination by noble gas mass spectrometry of {sup 22}Ne production through the combined reactions {sup 19}F({alpha},n){sup 22}Na({beta}{sup +}){sup 22}Ne and {sup 19}F({alpha},p){sup 22}Ne on natural calcium fluoride is made for the first time. Six samples of U-rich fluorite from a fluorspar deposit in Mexico were used to determine the {sup 22}Ne{sub nucl}/{sup 4}He{sub rad} ratio generated by the spontaneous decay of U during the last 32 Ma. The obtained ratio (1.33 {+-} 0.11) x10{sup -5} (95% confidence), is compared to other experimental data on natural uranium oxides and theoretical values.

  16. Vortex Shedding from an Object Moving in Superfluid ^4{He} at mK Temperatures and in a Bose-Einstein Condensate

    NASA Astrophysics Data System (ADS)

    Schoepe, W.

    2016-08-01

    Vortex shedding from a microsphere oscillating in superfluid ^4{He} at mK temperatures is compared with that from a laser beam moving in a Bose-Einstein condensate as observed by other authors. In particular, in either case a linear dependence of the shedding frequency f_v on Δ v = v - v_c is observed, where v is the velocity amplitude of the sphere or the constant velocity of the laser beam above a critical velocity v_c for the onset of turbulent flow: f_v = a Δ v , where the coefficient a is proportional to the oscillation frequency ω above some characteristic frequency ω _k and assumes a finite value for steady motion ω → 0.

  17. The halogen (F, Cl, Br, I) and H2O systematics of Samoan lavas: Assimilated-seawater, EM2 and high-3He/4He components

    NASA Astrophysics Data System (ADS)

    Kendrick, Mark A.; Jackson, Matthew G.; Hauri, Erik H.; Phillips, David

    2015-01-01

    The Samoan mantle plume samples two or more mantle components including an extreme EM2 composition with 87Sr/86Sr > 0.720 and a primitive component with high 3He/4He. The high 87Sr/86Sr melts have a unique potential to constrain the composition of the EM2 mantle end-member that is commonly attributed to subduction recycling. However, a previous study of H2O, CO2, S, F and Cl in Samoan glasses was hampered by the presence of unresolved assimilated sea water. The current study builds on the earlier work by extending the volatile database to include the trace halogens Br and I, and reporting new volatile data for additional glasses with 87Sr/86Sr up to 0.7125 and 3He/4He up to 15 Ra (Ra is the atmospheric 3He/4He ratio of 1.39 ×10-6). The selected glasses with MgO of 4.0 to 6.5 wt.% have CO2 concentrations of 4 to 200 ppm that reflect degassing of CO2 on the seafloor. The glasses contain 0.7-1.9 wt.% H2O, 880-1870 ppm F, 490-1790 ppm Cl, 1.9-7.2 ppm Br, 19-130 ppb I and 0.6-1.7 wt.% K. Correlations between the concentrations of these elements suggest the melts retain H2O concentrations close to pre-degassing values and demonstrate the melts have been variably affected by assimilation of seawater-derived brines. The brines are indicated to have had salinities of 55 ± 15 wt.% salt, F/Cl ratios close to seawater (e.g. <0.0001), Br/Cl ratios ∼ 40% higher than seawater, and I/Cl ratios ten times the seawater value. It is calculated the melts assimilated brine fractions of 0 to 0.45 wt.%, which contributed up to ∼30% of the total H2O and up to ∼70% of the total Cl in the melts. After accounting for the effects of brine assimilation, the Samoan melts are suggested to have a fairly constant magmatic Cl/K of 0.05 ± 0.2, which is lower than the median MORB value. Assimilation-corrected H2O/Ce values are not correlated with 87Sr/86Sr, but the sample with the highest 87Sr/86Sr of 0.7125 has an assimilation-corrected H2O/Ce of 83 ± 3, that is significantly lower than

  18. Primordial 4He abundance: a determination based on the largest sample of H II regions with a methodology tested on model H II regions

    NASA Astrophysics Data System (ADS)

    Izotov, Y. I.; Stasińska, G.; Guseva, N. G.

    2013-10-01

    We verified the validity of the empirical method to derive the 4He abundance used in our previous papers by applying it to CLOUDY (v13.01) models. Using newly published He i emissivities for which we present convenient fits as well as the output CLOUDY case B hydrogen and He i line intensities, we found that the empirical method is able to reproduce the input CLOUDY 4He abundance with an accuracy of better than 1%. The CLOUDY output data also allowed us to derive the non-recombination contribution to the intensities of the strongest Balmer hydrogen Hα, Hβ, Hγ, and Hδ emission lines and the ionisation correction factors for He. With these improvements we used our updated empirical method to derive the 4He abundances and to test corrections for several systematic effects in a sample of 1610 spectra of low-metallicity extragalactic H ii regions, the largest sample used so far. From this sample we extracted a subsample of 111 H ii regions with Hβ equivalent width EW(Hβ) ≥ 150 Å, with excitation parameter x = O2+/O ≥ 0.8, and with helium mass fraction Y derived with an accuracy better than 3%. With this subsample we derived the primordial 4He mass fraction Yp = 0.254 ± 0.003 from linear regression Y - O/H. The derived value of Yp is higher at the 68% confidence level (CL) than that predicted by the standard big bang nucleosynthesis (SBBN) model, possibly implying the existence of different types of neutrino species in addition to the three known types of active neutrinos. Using the most recently derived primordial abundances D/H = (2.60 ± 0.12) × 10-5 and Yp = 0.254 ± 0.003 and the χ2 technique, we found that the best agreement between abundances of these light elements is achieved in a cosmological model with baryon mass density Ωbh2 = 0.0234 ± 0.0019 (68% CL) and an effective number of the neutrino species Neff = 3.51 ± 0.35 (68% CL). Based on observations collected at the European Southern Observatory, Chile, programs 073.B-0283(A), 081.C-0113(A

  19. The 4He Total Photo-Absorption Cross Section With Two- Plus Three-Nucleon Interactions From Chiral Effective Field Theory

    SciTech Connect

    Quaglioni, S; Navratil, P

    2007-03-09

    The total photo-absorption cross section of {sup 4}He is evaluated microscopically using two- (NN) and three-nucleon (NNN) interactions based upon chiral effective field theory ({chi}EFT). The calculation is performed using the Lorentz integral transform method along with the ab initio no-core shell model approach. An important feature of the present study is the consistency of the NN and NNN interactions and also, through the Siegert theorem, of the two- and three-body current operators. This is due to the application of the {chi}EFT framework. The inclusion of the NNN interaction produces a suppression of the peak height and enhancement of the tail of the cross section. We compare to calculations obtained using other interactions and to representative experiments. The rather confused experimental situation in the giant resonance region prevents discrimination among different interaction models.

  20. Spin-polarized /sup 3/He nuclear targets and metastable /sup 4/He atoms by optical pumping with a tunable, Nd:YAP laser

    SciTech Connect

    Bohler, C.L.; Schearer, L.D.; Leduc, M.; Nacher, P.J.; Zachorowski, L.; Milner, R.G.; McKeown, R.D.; Woodward, C.E.

    1988-04-15

    Several Nd:YAP lasers were constructed which could be broadly tuned in the 1083-nm region which includes the helium 2/sup 3/S-2/sup 3/P transition, using a Lyot filter and thin, uncoated etalons within the laser cavity. 1 W of power could be extracted at 1083 nm through a 1% transmitting output coupler. This laser beam was used to optically pump metastable /sup 4/He and /sup 3/He 2/sup 3/S helium atoms in a weak discharge cell, spin polarizing the metastable ensemble. In a /sup 3/He cell the polarization is transferred to the nuclear spin system. A /sup 3/He target cell at 0.3 Torr was polarized to 52% in a few minutes. We describe the application of this system to the design of polarized targets for experiments in nuclear physics.

  1. Laser-spectroscopy measurement of the fine-structure splitting 2 3P1-2 3P2 of 4He

    NASA Astrophysics Data System (ADS)

    Feng, G.-P.; Zheng, X.; Sun, Y. R.; Hu, S.-M.

    2015-03-01

    Laser spectroscopy has been performed on a beam of neutral 4He atoms. By using transverse laser cooling and focusing, we are able to prepare a bright beam of atoms in the metastable state 2 3S1 deflected from the original effusive atomic beam. The initial state preparation is completed with optical pumping on the 2 3P1←2 3S1 transition at the wavelength of 1083 nm, followed by laser spectroscopy on the 2 3P1 ,2←2 3S1 transitions. The 2 3P1-2 3P2 fine-structure splitting is determined to be 2 291 177.69 ±0.36 kHz . The quantum interference effect is included in data extraction. This is the most precise laser spectroscopy measurement of the interval. Our result is in agreement with both the latest QED-based calculation and the most precise measurement conducted with microwave spectroscopy.

  2. A non-LTE spectral analysis of the 3He and 4He isotopes in the HgMn star κ Cancri

    NASA Astrophysics Data System (ADS)

    Maza, Natalia L.; Nieva, María-Fernanda; Przybilla, Norbert

    2014-12-01

    Aims: We present a pilot study on non-local thermodynamic equilibrium (NLTE) line-formation computations for the isotopes 3He and 4He in the mercury-manganese star κ Cancri. The impact of NLTE effects on the determination of isotopic abundances and the vertical stratification of helium in the atmosphere is investigated. Methods: Modern NLTE line-formation computations were employed to analyse a high-resolution and high signal-to-noise ratio ESO-VLT/UVES spectrum of κ Cnc. The atmospheric parameters were determined from fitting the hydrogen Balmer lines and the spectral energy distribution. Multiple He i lines were investigated, including He i λ4921 Å and λ6678 Å, which show the widest isotopic splits. Results: Half of the observed He i lines in the spectrum of κ Cnc show significant NLTE strengthening, the effects are strongest in the red lines He iλ5875 Å and He iλ6678 Å. NLTE abundances from individual He i lines are up to a factor of ~3 lower than LTE values. Helium is found to be stratified in the atmosphere of κ Cnc. While the LTE analysis indicates a step-like profile of the helium abundance, a gradual decrease with height is indicated by the NLTE analysis. A 3He/4He ratio of ~0.25-0.30 is found. With the available data it cannot be decided whether the two isotopes follow the same stratification profile, or not. Conclusions: This work implies that NLTE effects may be ubiquitous in the atmospheres of HgMn stars and may have a significant impact on abundance determinations and the interpretation of the vertical abundance stratification of elements. Based on data products from observations made with ESO Telescopes at the La Silla Paranal Observatory under programme ID 076.B-0055(A).Figures 3 and 4 are available in electronic form at http://www.aanda.org

  3. Autoradiographic 3H-Gaboxadol Receptor Binding Protocol

    PubMed Central

    Ling, Lynne; Caspary, Donald

    2016-01-01

    Gaboxadol (4,5,6,7-tetrahydroisoxazolo[5,4-c]pyridin-3-ol, THIP), a GABAA receptor δ-subunit specific agonist, when present at low (μM) concentrations, preferentially binds and activates extrasynaptic (non-γ2, δ-subunit-containing) GABAARs (Storustovu and Ebert, 2006; Richardson et al., 2011, 2013). In this prototype saturation binding experiment, a series of concentrations of [3H]gaboxadol (5, 10, 25, 50, 75, 100, 250 and 400 nM) will be used. GABA at 200 μM will be added into binding mixtures as a cold displacer for [3H]gaboxadol. Slide mailers are used and each requires 7 ml binding mixture. Pre-, post-washing and binding buffer is 50 mM Tris-Citrate (pH 7.1). The detailed procedure is outlined below.

  4. Astronomical identification of the C3H radical

    NASA Technical Reports Server (NTRS)

    Thaddeus, P.; Gottlieb, C. A.; Hjalmarson, A.; Johansson, L. E. B.; Irvine, W. M.

    1985-01-01

    The C3H radical has been identified in the millimeter-wave spectra of IRC +10216 and TMC-1. In IRC +10216, four rotational transitions have been observed, three in the lower fine-structure ladder (2Pi1/2) and one in the upper (2Pi3/2), each a resolved or partially resolved lambda-doublet. In TMC-1, both lambda components of the lowest lying 3/2-1/2 transition of the 2Pi1/2 ladder have been observed, each with well-resolved hfs. In IRC +10216, the excitation of C3H is similar to that of SiCC: the rotational temperature Trot within the 2Pi1/2 ladder is low (8.5 K), because of rapid radiative decay, while Trot across the ladders is high (about 52 K), because interconnecting far-IR radiative transitions are only weakly permitted. The column density of C3H in IRC +10216 averaged over the estimated source diameter of 84 arcsec is 2.8 x 10 to the 13th/sq cm, an order of magnitude less than that of C2H and C4H.

  5. (/sup 3/H)nitrendipine binding to adrenal capsular membranes

    SciTech Connect

    Finkel, M.S.; Aguilera, G.; Catt, K.J.; Keiser, H.R.

    1984-08-20

    The physiologic regulation of aldosterone secretion is dependent on extracellular calcium and appears to be mediated by increases in cytosolic free calcium concentration in the zona glomerulosa cell. A specific role for voltage-dependent calcium channels was suggested by previous studies with the calcium channel antagonist verapamil. The authors therefore studied the (/sup 3/H)nitrendipine calcium channel binding site in adrenal capsules. These studies revealed a single class of saturable, high affinity sites with K/sub D/ = .26 +/- .04 nM and B/sub max/ = 105 +/- 5.7 fmol/mg protein. Specific binding of (/sup 3/H)nitrendipine was inhibited by calcium channel antagonists with potencies nitrendipine = nifedipine >> verapamil, while diltiazem had no inhibitory effect. In the rat, binding sites for (/sup 3/H)nitrendipine were located in the adrenal capsule and medulla and were undetectable in the zona fasciculata. Physiologic studies with collagenase-dispersed adrenal glomerulosa cells demonstrated that nifedipine selectively inhibited angiotensin-II and potassium-stimulated steroidogenesis. These observations suggest both a pharmacologic and physiologic role for the nitrendipine binding site in aldosterone production. 17 references, 2 figures, 1 table.

  6. Evidence for a dynamically refracted primary bow in weakly bound 9Be rainbow scattering from 16O

    NASA Astrophysics Data System (ADS)

    Ohkubo, S.; Hirabayashi, Y.

    2016-09-01

    We present for the first time evidence for the existence of a dynamically refracted primary bow for 9Be+16O scattering. This is demonstrated through the use of coupled channel calculations with an extended double folding potential derived from the density-dependent effective two-body force and precise microscopic cluster wave functions for 9Be. The calculations reproduce the experimental Airy structure in 9Be+16O scattering well. It is found that coupling of a weakly bound 9Be nucleus to excited states plays the role of a booster lens, dynamically enhancing the refraction over the static refraction due to the Luneburg lens mean field potential between the ground states of 9Be and 16O.

  7. Relativity versus exchange currents in 16O(e ,e'p )

    NASA Astrophysics Data System (ADS)

    Grineviciute, J.; Halderson, Dean

    2016-07-01

    Background: The 16O(e ,e'p ) reaction in the quasielastic region has been studied in several experiments to determine spectroscopic factors, hence, the degree to which 16O looks like a closed shell. By varying the kinematics, experimentalists are able to extract response functions which comprise the cross section. However, analysis of the response functions separately produces very different spectroscopic factors. Two calculations led to different conclusions as to whether exchange currents can eliminate the discrepancies. Neither calculation considered relativistic corrections. Purpose: The purpose of the article is to investigate the disagreement as to whether exchange currents are the solution to obtaining consistent spectroscopic factors and to show that relativistic corrections have a much greater influence on providing this consistency. Methods: This calculation employs the recoil corrected continuum shell model, a model that uses a realistic interaction and produces nonspurious scattering states that are solutions to the coupled-channel problems. Pionic and pair contributions to the exchange currents were calculated as developed by Dubach et al. [Nucl. Phys. A 271, 279 (1976), 10.1016/0375-9474(76)90246-3]. Relativistic effects are included by use of the direct Pauli reduction. Results: Contributions of the exchange currents are shown to be insufficient to provide consistent spectroscopic factors. However, the inclusion of relativistic corrections produces spectroscopic factors from the different responses and cross sections which are very similar for both the p1 /2 and the p3 /2 states and both the (|q |,ω )=(460 MeV /c ,100 MeV ) and (|q |,ω )=(570 MeV /c ,172 MeV ) data. The influence of channel coupling is also shown to be significant. Tests of current conservation show that inclusion of the direct Pauli reduction produces small increases in its violation. Conclusions: Results are model dependent. Meson-exchange current contributions are not sufficient

  8. Effects of [3H]glucosamine concentration on [3H]chondroitin sulphate formation by cultured chondrocytes.

    PubMed Central

    Mroz, Paula J; Silbert, Jeremiah E

    2003-01-01

    GlcN (glucosamine) is now promoted over the counter for implied treatment of osteoarthritis, ostensibly by stimulating biosynthesis of cartilage chondroitin sulphate. In order to evaluate whether exogenous GlcN has any stimulatory effect, we have incubated mouse chondrocytes with [(35)S]sulphate and various amounts of GlcN, to determine whether any increment in chondroitin [(35)S]sulphate formation occurs. Similarly we have used varying concentrations of [(3)H]GlcN to determine the dilution of incorporation into [(3)H]chondroitin sulphate due to provision of endogenous GlcN by metabolism from glucose at two different glucose concentrations. The incorporation of both (35)S and (3)H was essentially linear over a 5 h time period. We found no stimulation of chondroitin [(35)S]sulphate synthesis at lower concentrations of GlcN, and a significant reduction at higher concentrations. Even at concentrations of [(3)H]GlcN that were greater than could be achieved with standard doses of oral GlcN, there was significant dilution of exogenous GlcN. Furthermore, an artificial acceptor for glycosaminoglycan synthesis in cell culture, 4-methylumbelliferyl beta-D-xyloside, did not modify the provision of GlcN from endogenous sources, even though it stimulated chondroitin sulphate synthesis 4 -5-fold at each GlcN concentration. We conclude that the cells have excess capacity to form maximal amounts of GlcN from glucose so that exogenous GlcN does not stimulate chondroitin sulphate synthesis. PMID:12943531

  9. Effect of sequence of administration on the pharmacokinetic interaction between the anticholinergic drug biperiden and [3H]quinuclidinyl benzylate or [3H]N-methylscopolamine in rats.

    PubMed

    Ishizaki, J; Yokogawa, K; Nakashima, E; Takayasu, T; Ohshima, T; Ichimura, F

    1998-02-01

    In rats the pharmacokinetic interactions between the anticholinergic drug biperiden and [3H]quinuclidinyl benzylate ([3H]QNB) or [3H]N-methylscopolamine ([3H]NMS) is affected by the sequence in which the drugs are administered. Drug concentrations in various tissues were determined after intravenous administration of [3H]QNB or [3H]NMS (325 ng kg(-1)). Biperiden (6.4 mg kg(-1)) was administered either 5 min before, concomitantly with or 20 min after injection of [3H]QNB or [3H]NMS. When biperiden was administered concomitantly with or before [3H]QNB, distribution of [3H]QNB among the regions of the brain and other tissues was reduced; at 4 h the ratio of the distribution of [3H]QNB for experimental animals to that for control animals ranged from 0.15 to 0.9. When biperiden was administered after [3H]QNB, the distribution of [3H]QNB in the brain and other tissues was significantly higher than for the other two treatments (P < 0.01). However, for [3H]NMS the sequence of administration had no effect on the distribution of the drug in the brain and other tissues except for the kidney. In-vitro, in crude synaptosomal membranes, the amount of [3H]QNB at 2 h relative to the control concentration at equilibrium was 87% when biperiden was added before [3H]QNB and 56% when biperiden was added after [3H]QNB. In both instances the concentration of [3H]NMS reached equilibrium within 30 min. These findings suggest that the difference between the rate constant of association and dissociation at the possible site of action gives rise to the effect of the sequence of administration on the pharmacokinetic interaction.

  10. Measurement of the Cascade Transition via the First Excited State of {sup 16}O in the {sup 12}C({alpha},{gamma}){sup 16}O Reaction, and Its S Factor in Stellar Helium Burning

    SciTech Connect

    Matei, C.; Brune, C. R.; Buchmann, L.; Hutcheon, D. A.; Caggiano, J.; Laird, A.; Li, ZH.; Olin, A.; Ottewell, D.; Ruprecht, G.; Trinczek, M.; Hannes, W. R.; Ruiz, C.; D'Auria, J.; Lamey, M.; Vockenhuber, C.; Wrede, C.; Chen, A. A.; Pearson, J.; Liu, WP.

    2006-12-15

    Radiative {alpha}-particle capture into the first excited, J{sup {pi}}=0{sup +} state of {sup 16}O at 6.049 MeV excitation energy has rarely been discussed as contributing to the {sup 12}C({alpha},{gamma}){sup 16}O reaction cross section due to experimental difficulties in observing this transition. We report here measurements of this radiative capture in {sup 12}C({alpha},{gamma}){sup 16}O for center-of-mass energies of E=2.22 MeV to 5.42 MeV at the DRAGON recoil separator. To determine cross sections, the acceptance of the recoil separator has been simulated in GEANT as well as measured directly. The transition strength between resonances has been identified in R-matrix fits as resulting both from E2 contributions as well as E1 radiative capture. Details of the extrapolation of the total cross section to low energies are then discussed [S{sub 6.0}(300)=25{sub -15}{sup +16} keV b] showing that this transition is likely the most important cascade contribution for {sup 12}C({alpha},{gamma}){sup 16}O.

  11. Energies of molecular structures in 12C,16O,20Ne,24Mg, and 32S

    NASA Astrophysics Data System (ADS)

    Royer, G.; Ramasamy, G.; Eudes, P.

    2015-11-01

    The energies of the 12C,16O,20Ne,24Mg, and 32S 4 n nuclei have been determined within a generalized liquid drop model and assuming different planar and three-dimensional shapes of the α molecules: linear chain, triangle, square, tetrahedron, pentagon, trigonal bipyramid, square pyramid, hexagon, octahedron, octagon, and cube. The potential barriers governing the entrance and decay channels via α absorption or emission as well as more symmetric binary and ternary reactions have been compared. The rms radii of the linear chains differ from the experimental rms radii of the ground states. The binding energies of the three-dimensional shapes at the contact point are higher than the ones of the planar configurations. The α particle plus A-4 daughter configuration leads always to the lowest potential barrier. The binding energy can be reproduced within the sum of the binding energy of n α particles plus the number of bonds multiplied by 2.4 MeV or by the sum of the binding energies of one α particle and the daughter nucleus plus the Coulomb energy and the proximity energy.

  12. Temporal pattern of incorporation of /sup 3/H precursors into pituitary glycoproteins and their subsequent release

    SciTech Connect

    Grotjan, H.E. Jr.

    1982-04-01

    The temporal pattern of incorporation of various /sup 3/H precursors into glycoproteins by rat anterior pituitaries incubated in vitro and the release of /sup 3/H-glycoproteins was examined. (/sup 3/H)Leucine incorporation was linear with respect to time and (/sup 3/H)leucine-containing macromolecules appeared in the media in about 1 hr. The temporal pattern of (/sup 3/H)mannose incorporation and release was similar. (/sup 3/H)Galactose and (/sup 3/H)fucose were incorporated after apparent time of delays of approximately 15 min and soon thereafter (20-25 min) appeared in the medium in /sup 3/H-glycoproteins. Thus, these precursors appear to be added as terminal residues. (/sup 3/H)Glucosamine exhibited a pattern intermediate between (/sup 3/H)leucine and (/sup 3/H)fucose whereas (/sup 3/H)GlcNAc appeared to be incorporated as a terminal residue.

  13. Interpretation of groundwater age tracers (CFC-12, 14C, 4He) in a mining-influenced stream-aquifer system with transient recharge dynamics.

    NASA Astrophysics Data System (ADS)

    Bourke, Sarah; Cook, Peter; Kipfer, Rolf; Dogramaci, Shawan

    2014-05-01

    Interpretation of groundwater age tracers often requires consideration of the mixing of groundwater with varying residence times. Quantification of mixing can be approached through measurement of multiple groundwater age indicators with varying ranges of temporal sensitivity, and their interpretation using lumped parameter models. However, in systems altered by mining, where recharge mechanisms are highly transient in space and time, lumped parameter models do not adequately represent the complexity of the system. In the Pilbara region of Western Australia, water abstracted during dewatering of ore-body aquifers is disposed of by discharging it into ephemeral streams and allowing it to recharge the aquifer. Because this water is essentially being recycled, stable isotopes and chloride are not useful tracers of the impact of this dewatering discharge. In contrast, gas tracers that respond rapidly to exposure to the atmosphere are more useful tracers for constraining the influence of dewatering discharge on the aquifer water balance. In this study we measured CFC-12, 14C and noble gases in production wells and transects of piezometers perpendicular to the stream. Even in samples from wells screened over intervals of 1 m, we observe combinations of tracer concentrations that indicate mixing of groundwater with contrasting residence times. For example, all samples contained measureable CFC-12 concentrations, including those with appreciable terrigenic 4He. Interpretation of these data requires consideration of the history of mining activity in the area. Stream 14C activities, which now range from 50 to 75 pMC, are a function of the dewatering discharge, and are no longer in equilibrium with the atmosphere. As a result, groundwater that recharged prior to mining operations can have higher 14C activities than groundwater that recharged through the stream in the last 10 years. The dewatering discharge has caused the stream to transition from a disconnected ephemeral

  14. Depth profiling of oxidized a-C:D Layers on Be -- A comparison of {sup 4}He RBS and {sup 28}Si ERD analysis

    SciTech Connect

    Roth, J.; Mayer, M.; Walsh, D.; Wampler, W.R.

    1997-06-01

    In applications dealing with the deposition of amorphous hydrogenated carbon layers or in the determination of the composition of deposited layers on the walls of nuclear fusion plasma experiments, the analysis of mixtures of light elements on heavy substrates is necessary. Depth profiling by means of RBS is often difficult due to the overlap of the backscattering intensities of different constituents from different depths. The erosion and reaction of deposited amorphous deuterated carbon (a-C:D) films with a Be substrate due to annealing in air poses an analytical challenge especially if simultaneously the exchange of hydrogen isotopes should be monitored. The analysis of the different recoiling atoms from collisions with heavy ions in Elastic Recoil Detection (ERD) can provide a tool which resolves all constituents in a single analysis. In the present study the composition of intermixed layers on Be containing H, D, Be, C and O has been analyzed using conventional {sup 4}He RBS at 2.2 MeV together with 2.5 MeV {sup 4}He ERD for hydrogen isotope analysis. At these energies, an overlap of signals from different constituents could be avoided in most cases. As alternative method heavy ion ERD using Si{sup 7+} ions extracted from a 5 MeV Tandem Van de Graff accelerator was investigated. At a scattering angle of 30{degree} Si ions could not be scattered into the detector and a solid state detector without protecting foil could be used. Even in the intermixed layers at terminal energies of 5 MeV the heavy constituents could be separated while signals from recoiling hydrogen and deuterium atoms could be resolved on top of the signal from the Be substrate. For the analysis of the RBS and ERD data the newly developed spectra simulation program SIMNRA has been used which includes a large data bank for scattering and nuclear reaction cross sections. The depth profiles of all constituents extracted from the simulation are compared for both methods.

  15. R-Matrix Evaluation of {sup 16}O neutron cross sections up to 6.3 MeV

    SciTech Connect

    Sayer, R.O.; Leal, L.C.; Larson, N.M.; Spencer, R.R.; and Wright, R.Q.

    2000-08-01

    In this paper the authors describe an evaluation of {sup 16}O neutron cross sections in the resolved resonance region with the multilevel Reich-Moore R-matrix formalism. Resonance analyses were performed with the computer code SAMMY [LA98] which utilizes Bayes' method, a generalized least squares technique.

  16. Comment on 'Low-energy cross sections in the {sup 12}C({alpha},{gamma}){sup 16}O reaction'

    SciTech Connect

    Descouvemont, P.; Dufour, M.

    2010-02-15

    We show that the E1 and E2 S factors recommended by Katsuma [Phys. Rev. C 78, 034606 (2008)] do not include well-known constraints and that the model is inappropriate for the {sup 12}C({alpha},{gamma}){sup 16}O reaction.

  17. Actinides produced by /sup 12/C + /sup 242/Pu and /sup 16/O + /sup 238/U reactions

    SciTech Connect

    Shinohara, N.; Usuda, S.; Ichikawa, S.; Suzuki, T.; Magara, M.; Okashita, H.; Yoshikawa, H.; Horiguchi, T.; Iwata, Y.; Shibata, S.; and others

    1986-09-01

    The cross sections for /sup 250/Fm, /sup 244-246/Cf, /sup 242-244/Cm, and /sup 242/Am/sup g-italic/ produced by the /sup 12/C+ /sup 242/Pu and the /sup 16/O+ /sup 238/U reactions leading to the same compound nucleus of /sup 254/Fm have been measured by using radiochemical methods. The excitation functions show that the difference between the /sup 12/C+ /sup 242/Pu and the /sup 16/O+ /sup 238/U reactions can be attributed mainly to the Coulomb barriers. Our results were compared with others reported previously for /sup 22/Ne+ /sup 232/Th, /sup 12/C+ /sup 238/U, /sup 12/C+ /sup 240,241/Pu, /sup 13/C+ /sup 241/Pu, /sup 16/O+ /sup 233/U, and /sup 16/O+ /sup 242/Pu reaction systems, and support a mechanism involving transfer of ..cap alpha..-particle clusters (C,Be,He) from projectile to target for the production of Cf and Cm isotopes.

  18. Effective theory of 3H and 3He

    NASA Astrophysics Data System (ADS)

    König, Sebastian; Grießhammer, Harald W.; Hammer, H.-W.; van Kolck, U.

    2016-06-01

    We present a new perturbative expansion for pionless effective field theory with Coulomb interactions in which at leading order (LO) the spin-singlet nucleon-nucleon channels are taken in the unitarity limit. Presenting results up to next-to-leading order for the Phillips line and the neutron-deuteron doublet-channel phase shift, we find that a perturbative expansion in the inverse {}1{S}0 scattering lengths converges rapidly. Using a new systematic treatment of the proton-proton sector that isolates the divergence due to one-photon exchange, we renormalize the corresponding contribution to the {}3{{H}} -{}3{He} binding energy splitting and demonstrate that the Coulomb force in pionless EFT is a completely perturbative effect in the trinucleon bound-state regime. In our new expansion, the LO is exactly isospin-symmetric. At next-to-leading order, we include isospin breaking via the Coulomb force and two-body scattering lengths, and find for the energy splitting {({E}B{(}3{He})-{E}B{(}3{{H}}))}{NLO}\\quad =(-0.86+/- 0.17)\\quad {MeV}.

  19. Beryllium-induced immune response in C3H mice

    SciTech Connect

    Benson, J.M.; Bice, D.E.; Nikula, K.J.

    1995-12-01

    Studies conducted at ITRI over the past several years have investigated whether Beagle dogs, monkeys, and mice are suitable models for human chronic beryllium-induced lung disease (CBD). Recent studies have focused on the histopathological and immunopathological changes occurring in A/J and C3H/HeJ mice acutely exposed by inhalation to Be metal. Lung lesions in both strains of mice included focal lymphocyte aggregates comprised primarily of B lymphocytes and lesser amounts of T-helper lymphocytes and microgranulomas consisting chiefly of macrophages and T-helper lymphocytes. The distribution of proliferating cells within the microgranulomas was similar to the distribution of T-helper cells. These results strongly suggested that A/J and C3H/HeJ mice responded to inhaled Be metal in a fashion similar to humans in terms of pulmonary lesions and the apparent in situ proliferation of T-helper cells. Results of these studies confirm lymphocyte involvement in the pulmonary response to inhaled Be metal.

  20. A search for interstellar oxiranecarbonitrile (C3H3NO).

    PubMed

    Dickens, J E; Irvine, W M; Ohishi, M; Arrhenius, G; Pitsch, S; Bauder, A; Muller, F; Eschenmoser, A

    1996-04-01

    We report a search in cold, quiescent and in 'hot core' type interstellar molecular clouds for the small cyclic molecule oxiranecarbonitrile (C3H3NO), which has been suggested as a precursor of important prebiotic molecules. We have determined upper limits to the column density and fractional abundance for the observed sources and find that, typically, the fractional abundance by number relative to molecular hydrogen of C3H3NO is less than a few times 10(-10). This limit is one to two orders of magnitude less than the measured abundance of such similarly complex species as CH3CH2CN and HCOOCH3 in well-studied hot cores. A number of astrochemical discoveries were made, including the first detection of the species CH3CH2CN in the massive star-forming clouds G34.3+0.2 and W51M and the first astronomical detections of some eight rotational transitions of CH3CH2CN, CH3CCH, and HCOOCH3. In addition, we found 8 emission lines in the 89 GHz region and 18 in the 102 GHz region which we were unable to assign.

  1. Effective theory of 3H and 3He

    NASA Astrophysics Data System (ADS)

    König, Sebastian; Grießhammer, Harald W.; Hammer, H.-W.; van Kolck, U.

    2016-06-01

    We present a new perturbative expansion for pionless effective field theory with Coulomb interactions in which at leading order (LO) the spin-singlet nucleon–nucleon channels are taken in the unitarity limit. Presenting results up to next-to-leading order for the Phillips line and the neutron–deuteron doublet-channel phase shift, we find that a perturbative expansion in the inverse {}1{S}0 scattering lengths converges rapidly. Using a new systematic treatment of the proton–proton sector that isolates the divergence due to one-photon exchange, we renormalize the corresponding contribution to the {}3{{H}} –{}3{He} binding energy splitting and demonstrate that the Coulomb force in pionless EFT is a completely perturbative effect in the trinucleon bound-state regime. In our new expansion, the LO is exactly isospin-symmetric. At next-to-leading order, we include isospin breaking via the Coulomb force and two-body scattering lengths, and find for the energy splitting {({E}B{(}3{He})-{E}B{(}3{{H}}))}{NLO}\\quad =(-0.86+/- 0.17)\\quad {MeV}.

  2. A Search for Interstellar Oxiranecarbonitrile (C3H3NO)

    NASA Technical Reports Server (NTRS)

    Dicken, J. E.; Irvine, W. M.; Ohishi, M.; Arrhenius, G.; Bauder, A.; Mueller, F.; Eschenmoser, A.

    1996-01-01

    We report a search in cold, quiescent and in 'hot core' type interstellar molecular clouds for the small cyclic molecule oxiranecarbonitrile (C3H3NO), which has been suggested as a precursor of important prebiotic molecules. We have determined upper limits to the column density and fractional abundance for the observed sources and find that, typically, the fractional abundance by number relative to molecular hydrogen Of C3H3NO is less than a few times 10(exp -10). This limit is one to two orders of magnitude less than the measured abundance of such similarly complex species as CH3CH2CN and HCOOCH3 in well-studied hot cores. A number of astrochemical discoveries were made, including the first detection of the species CH3CH2CN in the massive star-forming clouds G34.3+0.2 and W51M and the first astronomical detections of some eight rotational transitions of CH3CH2CN, CH3CCH, and HCOOCH3. In addition, we found 8 emission lines in the 89 GHz region and 18 in the 102 GHz region which we were unable to assign.

  3. Isotopically uniform, 16O-depleted calcium, aluminum-rich inclusions in CH and CB carbonaceous chondrites

    NASA Astrophysics Data System (ADS)

    Krot, Alexander N.; Nagashima, Kazuhide; Petaev, Michail I.

    2012-04-01

    In situ oxygen-isotope measurements of calcium-aluminum-rich inclusions (CAIs) from the metal-rich carbonaceous chondrites Isheyevo (CH/CB-like), Acfer 214 paired with Acfer 182 (CH), QUE 94411 paired with QUE 94627 (CBb), and Hammadah al Hamra 237 (CBb) revealed the presence of a common population of igneous, isotopically uniform, 16O-depleted inclusions: Δ17O (average ± 2 standard deviations) = -7 ± 4‰, -6 ± 5‰, and -8 ± 3‰, respectively. All CAIs from CBs and a significant fraction of those from CHs and Isheyevo are 16O-depleted. Most of the 16O-depleted CAIs consist of Ti-poor Al-diopside, spinel, melilite, and forsterite and surrounded by a single- and double-layered rim of forsterite ± diopside. The 16O-depleted CAIs composed of hibonite, grossite, melilite, and spinel, and surrounded by the multilayered melilite + diopside ± forsterite rims are less common. Some of the 16O-depleted refractory igneous inclusions composed of Al-diopside, forsterite, and ±spinel have chondrule-like textures (skeletal or barred). They are mineralogically most similar to Al-diopside-rich chondrules found in metal-rich carbonaceous chondrites and composed of Al-diopside, forsterite, Al-rich low-Ca pyroxene, ±glassy mesostasis, and ±spinel, suggesting there is a continuum between these objects. We suggest that (i) most of the isotopically uniform and 16O-depleted CAIs resulted from remelting of pre-existing, possibly 16O-rich refractory inclusions. The remelting may have occurred during formation of the magnesian, non-porphyritic (cryptocrystalline and skeletal) chondrules in CHs, CBs, and Isheyevo either by an unspecified, late, single-stage, highly-energetic event or in an impact-generated plume previously hypothesized for their origin; both mechanisms probably occurred in the solar nebula (i.e., in the presence of the nebula gas). The forsterite ± pyroxene rims around 16O-depleted CAIs may have resulted from evaporation-recondensation of silicon and magnesium

  4. 7Be (n ,α )4He Reaction and the Cosmological Lithium Problem: Measurement of the Cross Section in a Wide Energy Range at n_TOF at CERN

    NASA Astrophysics Data System (ADS)

    Barbagallo, M.; Musumarra, A.; Cosentino, L.; Maugeri, E.; Heinitz, S.; Mengoni, A.; Dressler, R.; Schumann, D.; Käppeler, F.; Colonna, N.; Finocchiaro, P.; Ayranov, M.; Damone, L.; Kivel, N.; Aberle, O.; Altstadt, S.; Andrzejewski, J.; Audouin, L.; Bacak, M.; Balibrea-Correa, J.; Barros, S.; Bécares, V.; Bečvář, F.; Beinrucker, C.; Berthoumieux, E.; Billowes, J.; Bosnar, D.; Brugger, M.; Caamaño, M.; Calviani, M.; Calviño, F.; Cano-Ott, D.; Cardella, R.; Casanovas, A.; Castelluccio, D. M.; Cerutti, F.; Chen, Y. H.; Chiaveri, E.; Cortés, G.; Cortés-Giraldo, M. A.; Cristallo, S.; Diakaki, M.; Domingo-Pardo, C.; Dupont, E.; Duran, I.; Fernandez-Dominguez, B.; Ferrari, A.; Ferreira, P.; Furman, W.; Ganesan, S.; García-Rios, A.; Gawlik, A.; Glodariu, T.; Göbel, K.; Gonçalves, I. F.; González-Romero, E.; Griesmayer, E.; Guerrero, C.; Gunsing, F.; Harada, H.; Heftrich, T.; Heyse, J.; Jenkins, D. G.; Jericha, E.; Katabuchi, T.; Kavrigin, P.; Kimura, A.; Kokkoris, M.; Krtička, M.; Leal-Cidoncha, E.; Lerendegui, J.; Lederer, C.; Leeb, H.; Lo Meo, S.; Lonsdale, S. J.; Losito, R.; Macina, D.; Marganiec, J.; Martínez, T.; Massimi, C.; Mastinu, P.; Mastromarco, M.; Mazzone, A.; Mendoza, E.; Milazzo, P. M.; Mingrone, F.; Mirea, M.; Montesano, S.; Nolte, R.; Oprea, A.; Pappalardo, A.; Patronis, N.; Pavlik, A.; Perkowski, J.; Piscopo, M.; Plompen, A.; Porras, I.; Praena, J.; Quesada, J.; Rajeev, K.; Rauscher, T.; Reifarth, R.; Riego-Perez, A.; Rout, P.; Rubbia, C.; Ryan, J.; Sabate-Gilarte, M.; Saxena, A.; Schillebeeckx, P.; Schmidt, S.; Sedyshev, P.; Smith, A. G.; Stamatopoulos, A.; Tagliente, G.; Tain, J. L.; Tarifeño-Saldivia, A.; Tassan-Got, L.; Tsinganis, A.; Valenta, S.; Vannini, G.; Variale, V.; Vaz, P.; Ventura, A.; Vlachoudis, V.; Vlastou, R.; Vollaire, J.; Wallner, A.; Warren, S.; Weigand, M.; Weiß, C.; Wolf, C.; Woods, P. J.; Wright, T.; Žugec, P.; n TOF Collaboration

    2016-10-01

    The energy-dependent cross section of the 7Be (n ,α )4He reaction, of interest for the so-called cosmological lithium problem in big bang nucleosynthesis, has been measured for the first time from 10 meV to 10 keV neutron energy. The challenges posed by the short half-life of 7Be and by the low reaction cross section have been overcome at n_TOF thanks to an unprecedented combination of the extremely high luminosity and good resolution of the neutron beam in the new experimental area (EAR2) of the n_TOF facility at CERN, the availability of a sufficient amount of chemically pure 7Be, and a specifically designed experimental setup. Coincidences between the two alpha particles have been recorded in two Si -7Be -Si arrays placed directly in the neutron beam. The present results are consistent, at thermal neutron energy, with the only previous measurement performed in the 1960s at a nuclear reactor. The energy dependence reported here clearly indicates the inadequacy of the cross section estimates currently used in BBN calculations. Although new measurements at higher neutron energy may still be needed, the n_TOF results hint at a minor role of this reaction in BBN, leaving the long-standing cosmological lithium problem unsolved.

  5. A dry 3He-4He dilution refrigerator for a transition edge sensor microcalorimeter spectrometer system mounted on a transmission electron microscope

    NASA Astrophysics Data System (ADS)

    Maehata, K.; Hara, T.; Ito, T.; Yamanaka, Y.; Tanaka, K.; Mitsuda, K.; Yamasaki, N. Y.

    2014-05-01

    A dry 3He-4He dilution refrigerator (DR) was developed for a superconducting transition edge sensor (TES) microcalorimeter installed on a transmission electron microscope. This system could be used for energy dispersive X-ray spectroscopy (EDS) with an excellent energy resolution. A Gifford-McMahon (GM)-type mechanical cryocooler was used as a pre-cooler for the DR to ensure liquid helium was not consumed during operation. To reduce sound and vibrations generated by the GM cryocooler, the DR was separated from the GM cryocooler in a split system. The TES microcalorimeter was glued onto the top of a copper rod referred to as the snout, which was attached to the mixing chamber of the DR. The cooling power in the mixing chamber was 30 μW at 105 mK. The lowest temperature in the mixing chamber was 74 mK, and that at top of the snout was 86 mK. An energy resolution of 7.6 eV full width at half maximum for Si Kα X-rays of 1.74 keV was obtained by TES microcalorimeter EDS performed with the transmission electron microscope.

  6. 3He Bilayer Film Adsorbed on Graphite Plated with a Bilayer of 4He: a New Frustrated 2D Magnetic System

    NASA Astrophysics Data System (ADS)

    Neumann, Michael; Nyéki, Ján; Cowan, Brian; Saunders, John

    2006-09-01

    The heat capacity and NMR response of a 3He bilayer adsorbed on graphite plated with a bilayer of 4He have been measured over the temperature range 1-80 mK. We find that the first 3He layer requires the presence of a 3He fluid overlayer before it solidifies. Solidification is completed at a total coverage close to 9.85 nm-2, On further increasing the coverage the heat capacity maximum grows from `antiferromagnetic-like' (AFM-like) to `ferromagnetic-like' (FM-like). On the other hand, when the 3He layer first solidifies, it has a low temperature saturation magnetisation corresponding to a significant fraction of full polarisation, and this increases with increasing coverage. Furthermore the effective exchange constant inferred from the high temperature magnetisation data is always ferromagnetic. The effective exchange constants inferred from the heat capacity and magnetisation are significantly larger than those observed in the second layer of pure 3He films adsorbed on bare graphite. Otherwise there are strong similarities in the coverage dependence of the heat capacity and magnetisation, providing fresh insights into how the magnetic ground state of such 2D magnets evolves as the frustration is tuned with increasing coverage.

  7. An Improved Reaction Rate Formulation for Charged-Particle Induced Thermonuclear Reaction of {sup 2}H(d,{gamma}){sup 4}He

    SciTech Connect

    Aziz, Azni Abdul; Yusof, Norhasliza; Idris, Mahirah; Kassim, Hasan Abu

    2011-03-30

    The reaction rate formula utilized in compilations such as the Nuclear Astrophysics Compilation of Reaction Rates (NACRE) uses low energy approximation due to temperatures in stars are in the region of a few keVs. Most nuclear reaction experiments were done in MeV range and the interior temperatures of massive stars are {approx}10{sup 9} K. Hence an improved formulation for calculating the nuclear reaction rate that is applicable to high temperatures is discussed in this work. The exact tunneling probability that is applicable for all energies is obtained by solving the Schroedinger equation. This yields an enhanced expression for the astrophysical S-factor for calculating the thermonuclear reaction rate at high temperature. The thermonuclear reaction rate from this work is applied to the {sup 2}H(d,{gamma}){sup 4}He reaction and is compared with the NACRE compilation. This improved reaction rate can be included in the nuclear reaction network in a Big Bang nucleosynthesis (BBN) code or a stellar nuclear network code.

  8. Bindings of /sup 3/H-prazosin and /sup 3/H-yohimbine to alpha adrenoceptors in the guinea-pig stomach

    SciTech Connect

    Taniguchi, T.; Nishikawa, H.

    1988-01-01

    Alpha adrenoceptor subtypes have been investigated by radioligand binding study in guinea-pig stomach using /sup 3/H-prazosin and /sup 3/H-yohimbine. The specific /sup 3/H-prazosin binding to guinea-pig stomach was saturable and of high affinity with a Bmax of 33 fmol/mg protein. Specific /sup 3/H-yohimbine binding to the tissue was also saturable and of high affinity with a Bmax of 150 fmol/mg protein. Adrenergic drugs competed for /sup 3/H-prazosin binding in order of prazosin > phentolamine > methoxamine > norepinephrine > clonidine > epinephrine > yohimbine. These drugs competed for /sup 3/H-yohimbine binding in order of yohimbine > phentolamine > clonidine > epinephrine > norepinephrine > prazosin > methoxamine. They also examined whether dopamine receptors exist in guinea-pig stomach, using radioligand binding study. Specific binding of /sup 3/H-spiperone, /sup 3/H-apomorphine, /sup 3/H-dopamine and /sup 3/H-domperidone was not detectable in the stomach. Dopaminergic drugs such as dopamine, haloperidol, domperidone and sulpiride competed for /sup 3/H-prazosin binding in order of haloperidol > domperidone > dopamine > sulpiride. Metoclopramide, sulpiride and dopamine competed for /sup 3/H-yohimbine binding in order of metoclopramide > sulpiride > dopamine.

  9. Microautoradiographic localisation of [3H]sucrose and [3H]mannitol in Robinia pseudoacacia pulvinar tissues during phytochrome-mediated nyctinastic closure.

    PubMed

    Moysset, L; Llambrich, E; López-Iglesias, C; Simón, E

    2006-11-01

    We have analysed the incorporation of [(3)H]sucrose and [(3)H]mannitol in pulvinar motor cells of Robinia pseudoacacia L. during phytochrome-mediated nyctinastic closure. Pairs of leaflets, excised 2 h after the beginning of the photoperiod, were fed with 50 mM [(3)H]sucrose or [(3)H]mannitol, irradiated with red (15 min) or far-red (5 min) light and placed in the dark for 2-3 h. Label uptake was measured in whole pulvini by liquid scintillation counting. The distribution of labelling in pulvinar sections was assessed by both light and electron microautoradiography. [(3)H]Sucrose uptake was twice that of [(3)H]mannitol incorporation in both red- and far-red-irradiated pulvini. In the autoradiographs, [(3)H]sucrose and [(3)H]mannitol labelling was localised in the area from the vascular bundle to the epidermis, mainly in vacuoles, cytoplasm, and cell walls. Extensor and flexor protoplasts displayed a different distribution of [(3)H]sucrose after red and far-red irradiation. Far-red light drastically reduced the [(3)H]sucrose incorporation in extensor protoplasts and caused a slight increase in internal flexor protoplasts. After red light treatment, no differences in [(3)H]sucrose labelling were found between extensor and flexor protoplasts. Our results indicate a phytochrome control of sucrose distribution in cortical motor cells and seem to rule out the possibility of sucrose acting as an osmoticum. PMID:17102931

  10. Using 16O/18O to Determine the Evolutionary History of the R Coronae Borealis Stars

    NASA Astrophysics Data System (ADS)

    Clayton, Geoffrey; Geballe, Tom; Welch, Douglas; Tisserand, Patrick

    2013-08-01

    Of the Galactic hydrogen-deficient carbon (HdC) and R Coronae Borealis (RCB) stars for which oxygen isotopic ratios can be measured, all of them show 16O/18O < 5, values that are orders of magnitude lower than measured in other stars (the Solar value is 500). This suggests that most if not all HdC and RCB stars are highly enriched in 18O. This is an important clue in determining the evolutionary pathways of HdC and RCB stars, for which two models have been proposed: the double degenerate (white dwarf (WD) merger), and the final helium-shell flash (FF). No overproduction of 18O is expected in the FF scenario. However, some RCB stars also show characteristics, such as 13C and Lithium, seen in FF stars. Therefore, we are conducting a survey all the RCB stars in the LMC and SMC for the characteristics of a WD merger or a FF. Most of the stars have been surveyed for 13C already and we plan to survey them for Lithium in the future. This proposal is to use Gemini/Flamingos-2 to survey all the stars, which are cool enough to show CO bands, for the presence of 18O near 2.3 micron. The Magellanic Clouds provide an unbiased, relatively complete sample of RCB stars which are at a known distance so their bolometric luminosities can be used in our stellar evolution models. This survey, combined with our models, will reveal the true fraction of RCB stars formed by each of the proposed scenarios.

  11. Using 16O/18O to Determine the Evolutionary History of the R Coronae Borealis Stars

    NASA Astrophysics Data System (ADS)

    Clayton, Geoffrey; Geballe, Tom; Welch, Douglas; Tisserand, Patrick

    2014-08-01

    All of the Galactic hydrogen-deficient carbon (HdC) and R Coronae Borealis (RCB) stars for which oxygen isotopic ratios can be measured, show 16O/18O < 5, values that are orders of magnitude lower than measured in other stars (the Solar value is 500). This suggests that most if not all HdC and RCB stars are highly enriched in 18O. This is an important clue to determining the evolutionary pathways of HdC and RCB stars, for which two models have been proposed: the double degenerate (white dwarf (WD) merger), and the final helium-shell flash (FF). No overproduction of 18O is expected in the FF scenario. However, some RCB stars also show characteristics, such as 13C and Lithium, seen in FF stars. Therefore, we are conducting a survey of all the RCB stars in the LMC and SMC for the characteristics of a WD merger or a FF. Most of the stars have been surveyed for 13C already, and we are also planning to survey them for Lithium. But no RCB star in the Magellanic Clouds has been observed for 18O. The Magellanic Clouds provide an unbiased, relatively complete sample of RCB stars which are at a known distance so their bolometric luminosities can be used in our stellar evolution models. This proposal is to use Gemini/Flamingos-2 to survey all of the Magellanic Cloud stars, which are cool enough to show CO bands, for the presence of 18O near 2.3 micron. This survey, combined with our stellar evolution models, will reveal the true fraction of RCB stars formed by each of the proposed scenarios.

  12. Pressure Effects on Product Channels of the Allyl Radical Reactions; C3H5+C3H5 and C3H5+CH3

    NASA Astrophysics Data System (ADS)

    Halpern, J. B.; N'Doumi, M.; Fahr, A.

    2011-12-01

    Relatively large hydrocarbon molecules (C4, C6 and larger) have been detected in several planetary environments. The mechanism for the formation of such large molecular species and detailed mechanism for their potential destruction are not well understood and are of considerable current interest. Previously we have studied the kinetics and product channels of small unsaturated hydrocarbon radical (C2 and C3s) reactions relevant to planetary atmospheric modeling. Reactions of C2 radicals (such as vinyl, H2CCH and ethynyl C2H) and C3 radicals (such as propargyl, HCCCH2) can affect the abundances of a large number of stable observable C3, C4, C5, C6 and larger molecules, including linear, aromatic and even poly aromatic molecules. Pressure-dependent product yields have been determined experimentally for the self- and cross-radical reactions performed at 298 K and at pressures between ~4 Torr (0.5 kPa) and 760 Torr (101 kPa). Final reaction products were quantitatively determined using a gas chromatograph with mass spectrometry/flame ionization detection (GC/MS/FID). In some cases complementary computational studies extended the pressure and temperature range of the experiments and provided valuable information on the complex reaction mechanisms. Theses studies provide a systematic framework so that important energetic and structural parameters for radical-radical reactions can be assessed. Here we report recent results for the allyl radical reactions H2CCCH3+ H2CCCH3 and H2CCCH3+CH3. For the allyl radical self-reaction, at high pressures the "head -to-head", combination channel forming 1,5-hexadiene is dominant with a combination/disproportionation = 1,5-hexadiene/propyne ratio of about 24 at 500 Torr (67 kPa, T=298K). At low pressures the ratio is substantially reduced to about 1.2 (at 0.3 kPa) and other major products are observed including allene, propene, 1-butene and propyne.

  13. Infrared Predissociation Spectroscopy of the Hydrocarbon Cations C_3H^+, C_2H^+, and C_3H_2^+

    NASA Astrophysics Data System (ADS)

    Brünken, Sandra; Lipparini, Filippo; Gauss, Jürgen; Stoffels, Alexander; Redlich, Britta; van der Meer, Lex; Berden, Giel; Oomens, Jos; Schlemmer, Stephan

    2016-06-01

    Reactive hydrocarbon cations play an important role in the astrochemistry of the interstellar medium, but spectroscopic data, needed for their identification in astronomical observations, is sparse. Here we report the first gas-phase vibrational spectra of the linear C_3H^+ (^1 Σ), the radical cation C_2H^+ (^3 Π), and the linear-/cyclic-C_3H_2^+ (^2 Π /^2A_1, resp.). Broadband spectra were recorded by Ne- and He-messenger infrared-predissociation (IR-PD) action spectroscopy in a cryogenic (4-11 K) ion trap instrument (FELion) in the 250-3500 {wn} range using a free electron laser and a MIR-OPO at the FELIX (Free-Electron Laser for Infrared eXperiments) laboratory. The band positions (determined with a precision of 1-2 wn) covering the C-H and C-C stretching as well as several bending modes are compared to high-level (CCSD(T) with large basis sets) quantum-chemical calculations with an emphasis on anharmonic effects and on the influence of the rare-gas messenger atom. The experimental and theoretical data provide a solid basis for subsequent IR high-resolution studies, with the ultimate goal to predict and measure accurate rotational spectra for a radio-astronomical search of these molecular ions in space.

  14. Encapsulated scintillators monitor /sup 3/H-solute concentrations

    SciTech Connect

    Kirk, G.; Gruner, S.

    1982-02-01

    The short range of the /sup 3/H beta allows shielding of microbeds of scintillator by a several um thick coating of a water based gel. Gels may be used which are permeable to a wide variety of tritiated molecules. Thus, the light output of a mixture of the coated beads and a solution of the tritiated compound is proportional to the solution concentration of the tritiated substance. The mixture may also contain particles to which the gel is impermeable, such as cells, vesicles, large proteins, etc., but which can alter the concentration of the tritiated compound by uptake or release. In this case, the light output monitors the fractional uptake of the tritiated material. The design criteria for encapsulating the scintillators and dynamically monitoring the scintillation output are discussed. A simple method for encapsulating plastic scintillator microbeads, suitable for monitoring slow concentration changes, is described and tested.

  15. One dimensional 1H, 2H and 3H

    NASA Astrophysics Data System (ADS)

    Vidal, A. J.; Astrakharchik, G. E.; Vranješ Markić, L.; Boronat, J.

    2016-05-01

    The ground-state properties of one-dimensional electron-spin-polarized hydrogen 1H, deuterium 2H, and tritium 3H are obtained by means of quantum Monte Carlo methods. The equations of state of the three isotopes are calculated for a wide range of linear densities. The pair correlation function and the static structure factor are obtained and interpreted within the framework of the Luttinger liquid theory. We report the density dependence of the Luttinger parameter and use it to identify different physical regimes: Bogoliubov Bose gas, super-Tonks-Girardeau gas, and quasi-crystal regimes for bosons; repulsive, attractive Fermi gas, and quasi-crystal regimes for fermions. We find that the tritium isotope is the one with the richest behavior. Our results show unambiguously the relevant role of the isotope mass in the properties of this quantum system.

  16. Measurement of the D/H, 18O/16O, and 17O/16O Isotope Ratios in Water by Laser Absorption Spectroscopy at 2.73 μm

    PubMed Central

    Wu, Tao; Chen, Weidong; Fertein, Eric; Masselin, Pascal; Gao, Xiaoming; Zhang, Weijun; Wang, Yingjian; Koeth, Johannes; Brückner, Daniela; He, Xingdao

    2014-01-01

    A compact isotope ratio laser spectrometry (IRLS) instrument was developed for simultaneous measurements of the D/H, 18O/16O and 17O/16O isotope ratios in water by laser absorption spectroscopy at 2.73 μm. Special attention is paid to the spectral data processing and implementation of a Kalman adaptive filtering to improve the measurement precision. Reduction of up to 3-fold in standard deviation in isotope ratio determination was obtained by the use of a Fourier filtering to remove undulation structure from spectrum baseline. Application of Kalman filtering enables isotope ratio measurement at 1 s time intervals with a precision (<1‰) better than that obtained by conventional 30 s averaging, while maintaining a fast system response. The implementation of the filter is described in detail and its effects on the accuracy and the precision of the isotope ratio measurements are investigated. PMID:24854363

  17. RCNP E398 {sup 16}O,{sup 12}C(p,p’) experiment: Measurement of the γ-ray emission probability from giant resonances in relation to {sup 16}O,{sup 12}C(ν,ν’) reactions

    SciTech Connect

    Ou, I.; Yamada, Y.; Mori, T.; Yano, T.; Sakuda, M.; Tamii, A.; Suzuki, T.; Yosoi, M.; Aoi, N.; Ideguchi, E.; Hashimoto, T.; Miki, K.; Ito, T.; Iwamoto, C.; Yamamoto, T.; Akimune, H.

    2015-05-15

    We propose to measure the γ-ray emission probability from excited states above 5 MeV including giant resonance of {sup 16}O and {sup 12}C as a function of excitation energy in 1-MeV step. Here, we measure both the excitation energy (E{sub x}=5-30MeV) at the forward scattering angles (0°-3°) of the {sup 16}O, {sup 12}C (p, p’) reaction using Grand-Raiden Spectrometer and the energy of γ-rays (E{sub γ}) using an array of NaI(Tl) counters. The purpose of the experiment is to provide the basic and important information not only for the γ-ray production from primary neutral-current neutrino-oxygen (-carbon) interactions but also for that from the secondary hadronic (neutron-oxygen and -carbon) interactions.

  18. Major and trace element composition of the high 3He/4He mantle: Implications for the composition of a nonchonditic Earth

    NASA Astrophysics Data System (ADS)

    Jackson, Matthew G.; Jellinek, A. Mark

    2013-08-01

    The bulk composition of the silicate portion of the Earth (BSE) has long been assumed to be tied to chondrites, in which refractory, lithophile elements like Sm and Nd exist in chondritic relative abundances. However, the 142Nd/144Nd ratios of modern terrestrial samples are 18 ± 5 ppm higher than the ordinary-chondrite reservoir, and this challenges the traditional BSE model. Here we investigate a hypothesis that this terrestrial 142Nd excess is related to a Sm/Nd ratio 6% higher than chondritic. This Sm/Nd ratio yields a superchondritic 143Nd/144Nd (˜0.5130) similar to that identified in the highest 3He/4He mantle reservoir, and we argue that this reservoir represents the BSE composition for lithophile elements. We develop a compositional model for BSE in which the elevated Sm/Nd requires a shift of 143Nd/144Nd from 0.51263 (chondritic) to 0.51300. The new BSE composition is depleted in highly incompatible elements, including K, relative to the chondrite-based BSE, and offers a solution the "missing" 40Ar paradox. This BSE compositional model requires that >83% of the mantle is depleted to form continental crust. It also implies a ˜30% reduction in BSE U, Th and K, and therefore in the current rate of radiogenic heating and, thus, a proportional increase in the heat flow delivered to surface by plate tectonics. We explore thermal history models including effects related to a newly recognized evolution in the style of plate tectonics over Earth history: The lower radiogenic heat production may delay the onset of core convection and dynamo action to as late as 3.5 Gyr.

  19. A transition-edge-sensor-based instrument for the measurement of individual He2* excimers in a superfluid 4He bath at 100 mK

    NASA Astrophysics Data System (ADS)

    Carter, Faustin Wirkus

    This dissertation is an account of the first calorimetric detection of individual He*2 excimers within a bath of superfluid 4He. When superfluid helium is subject to ionizing radiation, diatomic He molecules are created in both the singlet and triplet states. The singlet He molecules decay within nanoseconds, but due to a forbidden spin-flip the triplet molecules have a relatively long lifetime of 13 seconds in superfluid He. When He* 2 molecules decay, they emit a ~15 eV photon. Nearly all matter is opaque to these vacuum-UV photons, although they do propagate through liquid helium. The triplet state excimers propagate ballistically through the superfluid until they quench upon a surface; this process deposits a large amount of energy into the surface. The prospect of detecting both excimer states is the motivation for building a detector immersed directly in the superfluid bath. The detector used in this work is a single superconducting titanium transition edge sensor (TES). The TES is mounted inside a hermetically sealed chamber at the baseplate of a dilution refrigerator. The chamber contains superfluid helium at 100 mK. Excimers are created during the relaxation of high-energy electrons, which are introduced into the superfluid bath either in situ via a sharp tungsten tip held above the field-emission voltage, or by using an external gamma-ray source to ionize He atoms. These excimers either propagate through the LHe bath and quench on a surface, or decay and emit vacuum-ultraviolet photons that can be collected by the detector. This dissertation discusses the design, construction, and calibration of the TES-based excimer detecting instrument. It also presents the first spectra resulting from the direct detection of individual singlet and triplet helium excimers.

  20. Clinical and treatment effects on /sup 3/H-clonidine and /sup 3/H-imipramine binding in elderly depressed patients

    SciTech Connect

    Georgotas, A.; Schweitzer, J.; McCue, R.E.; Armour, M.; Friedhoff, A.J.

    1987-06-01

    /sup 3/H-clonidine and /sup 3/H-imipramine binding were measured in depressed patients, 55 years and older. There was no significant difference in either /sup 3/H-clonidine or /sup 3/H-imipramine binding between depressed patients and age- and sex-matched controls. There was no significant correlation between /sup 3/H-clonidine or /sup 3/H-imipramine binding and severity of depression before treatment. There was a significant negative correlation between the K/sub D/ of /sup 3/H-imipramine binding sites and Hamilton score over seven weeks of antidepressant treatment. There was no significant difference between receptor data of responders and nonresponders to antidepressant treatment. 19 references, 2 tables.

  1. Selective labeling of serotonin uptake sites in rat brain by (/sup 3/H)citalopram contrasted to labeling of multiple sites by (/sup 3/H)imipramine

    SciTech Connect

    D'Amato, R.J.; Largent, B.L.; Snowman, A.M.; Snyder, S.H.

    1987-07-01

    Citalopram is a potent and selective inhibitor of neuronal serotonin uptake. In rat brain membranes (/sup 3/H)citalopram demonstrates saturable and reversible binding with a KD of 0.8 nM and a maximal number of binding sites (Bmax) of 570 fmol/mg of protein. The drug specificity for (/sup 3/H)citalopram binding and synaptosomal serotonin uptake are closely correlated. Inhibition of (/sup 3/H)citalopram binding by both serotonin and imipramine is consistent with a competitive interaction in both equilibrium and kinetic analyses. The autoradiographic pattern of (/sup 3/H)citalopram binding sites closely resembles the distribution of serotonin. By contrast, detailed equilibrium-saturation analysis of (/sup 3/H)imipramine binding reveals two binding components, i.e., high affinity (KD = 9 nM, Bmax = 420 fmol/mg of protein) and low affinity (KD = 553 nM, Bmax = 8560 fmol/mg of protein) sites. Specific (/sup 3/H)imipramine binding, defined as the binding inhibited by 100 microM desipramine, is displaced only partially by serotonin. Various studies reveal that the serotonin-sensitive portion of binding corresponds to the high affinity sites of (/sup 3/H)imipramine binding whereas the serotonin-insensitive binding corresponds to the low affinity sites. Lesioning of serotonin neurons with p-chloroamphetamine causes a large decrease in (/sup 3/H)citalopram and serotonin-sensitive (/sup 3/H)imipramine binding with only a small effect on serotonin-insensitive (/sup 3/H)imipramine binding. The dissociation rate of (/sup 3/H)imipramine or (/sup 3/H)citalopram is not altered by citalopram, imipramine or serotonin up to concentrations of 10 microM. The regional distribution of serotonin sensitive (/sup 3/H)imipramine high affinity binding sites closely resembles that of (/sup 3/H)citalopram binding.

  2. 3,4-Methylenedioxyamphetamine (MDA) analogues exhibit differential effects on synaptosomal release of 3H-dopamine and 3H-5-hydroxytryptamine

    SciTech Connect

    McKenna, D.J.; Guan, X.M.; Shulgin, A.T. )

    1991-03-01

    The effect of various analogues of the neurotoxic amphetamine derivative, MDA (3,4-methylenedioxyamphetamine) on carrier-mediated, calcium-independent release of 3H-5-HT and 3H-DA from rat brain synaptosomes was investigated. Both enantiomers of the neurotoxic analogues MDA and MDMA (3,4-methylenedioxymethamphetamine) induce synaptosomal release of 3H-5-HT and 3H-DA in vitro. The release of 3H-5-HT induced by MDMA is partially blocked by 10(-6) M fluoxetine. The (+) enantiomers of both MDA and MDMA are more potent than the (-) enantiomers as releasers of both 3H-5-HT and 3H-DA. Eleven analogues, differing from MDA with respect to the nature and number of ring and/or side chain substituents, also show some activity in the release experiments, and are more potent as releasers of 3H-5-HT than of 3H-DA. The amphetamine derivatives {plus minus}fenfluramine, {plus minus}norfenfluramine, {plus minus}MDE, {plus minus}PCA, and d-methamphetamine are all potent releasers of 3H-5-HT and show varying degrees of activity as 3H-DA releasers. The hallucinogen DOM does not cause significant release of either 3H-monoamine. Possible long-term serotonergic neurotoxicity was assessed by quantifying the density of 5-HT uptake sites in rats treated with multiple doses of selected analogues using 3H-paroxetine to label 5-HT uptake sites. In the neurotoxicity study of the compounds investigated, only (+)MDA caused a significant loss of 5-HT uptake sites in comparison to saline-treated controls. These results are discussed in terms of the apparent structure-activity properties affecting 3H-monoamine release and their possible relevance to neurotoxicity in this series of MDA congeners.

  3. Effectiveness of the statistical potential in the description of fermions in a worm-algorithm path-integral Monte Carlo simulation of 3He atoms placed on a 4He layer adsorbed on graphite.

    PubMed

    Ghassib, Humam B; Sakhel, Asaad R; Obeidat, Omar; Al-Oqali, Amer; Sakhel, Roger R

    2012-01-01

    We demonstrate the effectiveness of a statistical potential (SP) in the description of fermions in a worm-algorithm path-integral Monte Carlo simulation of a few 3He atoms floating on a 4He layer adsorbed on graphite. The SP in this work yields successful results, as manifested by the clusterization of 3He, and by the observation that the 3He atoms float on the surface of 4He. We display the positions of the particles in 3D coordinate space, which reveal clusterization of the 3He component. The correlation functions are also presented, which give further evidence for the clusterization.

  4. Quasielastic knockout of light fragments from {sup 12}C and {sup 16}O nuclei by intermediate-energy pions

    SciTech Connect

    Abramov, B. M.; Borodin, Yu. A.; Bulychjov, S. A.; Dukhovskoy, I. A.; Krutenkova, A. P.; Kulikov, V. V. Martemianov, M. A.; Matsuk, M. A.; Tarasov, V. E.; Turdakina, E. N.; Khanov, A. I.

    2007-07-15

    Quasielastic deuteron and triton knockout from {sup 12}C and {sup 16}O nuclei has been studied infull kinematics using a 0.72-GeV/c pion beam. The momentum distributions of the intranuclear quasideuteron motion, excitation-energy spectra of the residual nuclei, and the effective numbers N{sub d}{sup eff} of quasideuterons are determined. The parameters of the quasideuteron intranuclear motion are in reasonable agreement with the results obtained in other beams. The N{sub d}{sup eff} in the nuclei from {sup 6}Li to {sup 16}O measured in full kinematics are virtually independent of the atomic number in contrast to the analogous values in the inclusive deuteron-knockout reaction induced by protons. The phenomenon of triton knockout from these nuclei is observed, which makes possible estimation of the cross section of backward pion-triton elastic scattering in yet unexplored regions of energy and momentum transfer.

  5. Low-energy cross sections in the {sup 12}C({alpha},{gamma}){sup 16}O reaction

    SciTech Connect

    Katsuma, M.

    2008-09-15

    The low-energy {sup 12}C({alpha},{gamma}){sup 16}O reaction is analyzed with the potential model. The potentials are chosen from the deep potential describing the {alpha}-particle nuclear rainbow phenomena at high energies. Below E{sub c.m.}=1 MeV, the cross section is found to be dominated by the E2 transition to the ground state of {sup 16}O. No enhancement of the E1 component at low energies is predicted. The extrapolated astrophysical S-factors at E{sub c.m.}=0.3 MeV are S{sub E2}=150 keV b and S{sub E1}=3 keV b.

  6. The role of primary 16O as a neutron poison in AGB stars and fluorine primary production at halo metallicities.

    NASA Astrophysics Data System (ADS)

    Gallino, R.; Bisterzo, S.; Cristallo, S.; Straniero, O.

    The discovery of a historical bug in the s-post-process AGB code obtained so far by the Torino group forced us to reconsider the role of primary 16O in the 13C-pocket, produced by the 13C(alpha , n)16O reaction, as important neutron poison for the build up of the s-elements at Halo metallicities. The effect is noticeable only for the highest 13C-pocket efficiencies (cases ST*2 and ST). For Galactic disc metallicities, the bug effect is negligible. A comparative analysis of the neutron poison effect of other primary isotopes (12C, 22Ne and its progenies) is presented. The effect of proton captures, by 14N(n, p)14C, boosts a primary production of fluorine in halo AGB stars, with [F/Fe] comparable to [C/Fe], without affecting the s-elements production.

  7. Improved Data Set for the Herzberg Band Systems of 16O 2

    NASA Astrophysics Data System (ADS)

    Mérienne, Marie-France; Jenouvrier, Alain; Coquart, Bernard; Carleer, Michel; Fally, Sophie; Colin, Reginald; Vandaele, A. C.; Hermans, Christian

    2001-05-01

    Total number of files: 3+README.TXT Filenames: O2_HERZB.TXT NON_ATT.TXT O2_PARAM.TXT Filetypes: ASCII I-O2_HERZB.TXT The assignments and intensities in the 41261-34000 cm-1 region include the data from ref.1 and 2, and additional data from revisited spectra (ref.3). 1-FOURIER TRANSFORM SPECTROSCOPY OF THE O2 HERZBERG BANDS I. ROTATIONAl ANALYSIS A. Jenouvrier, M-F. Merienne, B. Coquart, M. Carleer, S. Fally, A.C. Vandaele, C. Hermans and R. Colin Journal of Molecular Spectroscopy 198,136-162 (1999) 2-FOURIER TRANSFORM SPECTROSCOPY OF THE O2 HERZBERG BANDS II. BAND OSCILLATOR STRENGTHS AND TRANSITION MOMENTS M-F. Merienne, A. Jenouvrier, B. Coquart, M. Carleer, S. Fally, R. Colin, A.C. Vandaele and C. Hermans Journal of Molecular Spectroscopy 202, 171-193 (2000) 3-IMPROVED DATA SET FOR THE HERZBERG BAND SYSTEMS OF {16}O2 M-F. Merienne, A. Jenouvrier, B. Coquart, M. Carleer, S. Fally, R. Colin, A.C. Vandaele and C. Hermans Journal of Molecular Spectroscopy DESCRIPTION: Columns: 1-Wavenumber in cm-1. 'c' denotes a calculated value for a blended line. 2-Integrated line cross section in 10-26 cm2 cm-1 molecule-1. '*' denotes a saturated line for which the value has been calculated. 3-Assignment in the order : electronic transition, vibrational band v'-0, branch, rotational assignment (N"). For the overlapped lines, the value in [ ] is the estimated integrated cross section. II-NON_ATT.TXT Lines which cannot be identified as {16}O2 transitions. DESCRIPTION: Columns: 1-Wavenumber in cm-1. 2-Integrated line cross section in 10-26 cm2 cm-1 molecule-1. III-O2_PARAM.TXT This file contains tables for the molecular parameters and the transition moments. table 1: A(3)Sigma(u)+ parameters (in cm-1): the numbers in parentheses are two standard deviations (2sigma) in units of the last digits. DESCRIPTION: Columns: 1-Vibrational quantum number v. 2-Band origin T(v) referred to the hypothetical X(3)Sigma(g)-, F2, N = J = 0 level. 3-Rotational constant B(v). 4-Rotational centrifugal

  8. New decay branches of the radiative capture reaction {sup 12}C({sup 16}O,{gamma}){sup 28}Si

    SciTech Connect

    Lebhertz, D.; Courtin, S.; Haas, F.; Salsac, M.-D.; Beck, C.; Michalon, A.; Rousseau, M.; Marley, P. L.; Glover, R. G.; Kent, P. E.; Hutcheon, D. A.; Davis, C.; Pearson, J. E.

    2009-01-28

    Resonances in the {sup 12}C({sup 16}O,{gamma}){sup 28}Si radiative capture process at energies around the Coulomb barrier have been probed using the very selective 0 deg. Dragon spectrometer at Triumf and its associated BGO {gamma}-array. For the first time the full level scheme involved in this process has been measured and shows previously unobserved {gamma}-decay to doorway states around 11 MeV in {sup 28}Si.

  9. CAF-1-induced oligomerization of histones H3/H4 and mutually exclusive interactions with Asf1 guide H3/H4 transitions among histone chaperones and DNA.

    PubMed

    Liu, Wallace H; Roemer, Sarah C; Port, Alex M; Churchill, Mair E A

    2012-12-01

    Anti-silencing function 1 (Asf1) and Chromatin Assembly Factor 1 (CAF-1) chaperone histones H3/H4 during the assembly of nucleosomes on newly replicated DNA. To understand the mechanism of histone H3/H4 transfer among Asf1, CAF-1 and DNA from a thermodynamic perspective, we developed and employed biophysical approaches using full-length proteins in the budding yeast system. We find that the C-terminal tail of Asf1 enhances the interaction of Asf1 with CAF-1. Surprisingly, although H3/H4 also enhances the interaction of Asf1 with the CAF-1 subunit Cac2, H3/H4 forms a tight complex with CAF-1 exclusive of Asf1, with an affinity weaker than Asf1-H3/H4 or H3/H4-DNA interactions. Unlike Asf1, monomeric CAF-1 binds to multiple H3/H4 dimers, which ultimately promotes the formation of (H3/H4)(2) tetramers on DNA. Thus, transition of H3/H4 from the Asf1-associated dimer to the DNA-associated tetramer is promoted by CAF-1-induced H3/H4 oligomerization.

  10. (/sup 3/H)U-69593 labels a subtype of kappa opiate receptor with characteristics different from that labeled by (/sup 3/H)ethylketocyclazocine

    SciTech Connect

    Nock, B.; Rajpara, A.; O'Connor, L.H.; Cicero, T.J.

    1988-01-01

    (/sup 3/H)U-69593 is an opiate agonist that has been reported to bind in vitro with high affinity and selectivity to the kappa receptor subtype. The studies reported here were designed to determine the optimal conditions for labeling kappa receptors with (/sup 3/H)U-69593 and to further characterize the binding site. The effects of temperature and NaCl on (/sup 3/H)U-69593 binding were of particular interest because previous studies reported that (/sup 3/H)ethylketocyclazocine ((/sup 3/H)EKC) and (/sup 3/H)bremazocine binding to kappa receptors was optimal at 4/sup 0/C in the presence of NaCl. Those conditions were not found to be optimal for (/sup 3/H)U-69593 binding. Although the pharmacological specificity and Bmax of (/sup 3/H)U-69593 binding was similar at room temperature and at 4/sup 0/C, the binding affinity was approximately three times lower at 4/sup 0/C than at room temperature. In addition, NaCl had an effect on (/sup 3/H)U-69593 binding that was opposite that on (/sup 3/H)EKC binding at 4/sup 0/C. These differences between (/sup 3/H)U-69593 and (/sup 3/H)EKC binding at 4/sup 0/C were accentuated by a vast difference in the density of the binding sites and suggested that (/sup 3/H)U-69593 might bind selectively to a kappa receptor subtype.

  11. In vivo labeling of cocaine receptors with sup 3 H-(-) cocaine, sup 3 H-WIN 35,065-2 and sup 3 H-WIN 35,428

    SciTech Connect

    Scheffel, U.; Boja, J.W.; Stathis, M.; Kuhar, M.J. )

    1990-02-26

    {sup 11}C-(-)cocaine (-COC) has recently been employed to image -COC binding sites in vivo using PET. Two analogs of -COC, WIN 35,065-2 (WIN-2) and WIN 35,428 (CFT), have been shown in vitro to exhibit higher affinity for the -COC receptor than -COC. The present study evaluates {sup 3}H-WIN-2 and {sup 3}H-CFT as in vivo receptor labels in mice with a view towards the use of these compounds as PET ligands for -COC receptors in the living human brain. {sup 3}H-labeled -COC, WIN-2 and CFT were injected i.v. into mice and their specific binding in the CNS determined. Peak striatal/cerebellar (S/C) ratios were reached at 5 minutes post injection with -COC (1.56), at 45 minutes with {sup 3}H-WIN-2 (3.30) and 60 minutes with {sup 3}H-CFT (4.0). The specificity of in vivo binding of {sup 3}H-WIN-2 and {sup 3}H-CFT was tested by pre-injection of various drugs. Binding of {sup 3}H-WIN-2 and {sup 3}H-CFT was dose-dependently blocked by cold WIN-2 and CFT, and by dopamine uptake site inhibitors (mazindol, GBR 12,909, nomifensine), but not by (+)COC, paroxetine and desipramine. The data indicate that {sup 3}H-WIN-2 and {sup 3}H-CFT exhibit improved in vivo binding (higher S/C ratios, longer retention time at the -COC receptor/dopamine transporter) compared to -COC and support their testing in PET studies.

  12. Elastic deuteron scattering on {sup 12}C and {sup 16}O nuclei in the alpha-cluster model

    SciTech Connect

    Berezhnoy, Yu. A.; Mikhailyuk, V. P.; Pilipenko, V. V. Fedorchenko, D. V.

    2013-07-15

    On the basis of the dispersive alpha-cluster model for target nuclei and the theory of multiple diffractive scattering, differential cross sections and analyzing powers for the elastic scattering of 400 and 700-MeV deuterons on {sup 12}C and {sup 16}O target nuclei were calculated in the pointlike-deuteron approximation. In these calculations, the amplitude for incident-deuteron scattering on nuclei was constructed with the aid of amplitudes for d{alpha} scattering that were obtained from a fit to data on d{sup 16}O scattering. The same features were calculated on the basis of the diffraction approximation with allowance for the internal deuteron structure by using the amplitudes obtained earlier for nucleon scattering on {sup 12}C and {sup 16}O nuclei within the same dispersive alpha-clustermodel. The latter made it possible to perform calculations without employing adjustable parameters. The observables calculated on the basis of either approach agree with available experimental data.

  13. Reactivity Impact of 2H and 16O Elastic Scattering Nuclear Data on Critical Systems with Heavy Water

    NASA Astrophysics Data System (ADS)

    Roubtsov, D.; Kozier, K. S.; Chow, J. C.; Plompen, A. J. M.; Kopecky, S.; Svenne, J. P.; Canton, L.

    2014-04-01

    The accuracy of deuterium nuclear data is important for reactor physics simulations of heavy water (D2O) reactors. The elastic neutron scattering cross section data at thermal energies, σs,th, have been observed to have noticeable impact on the reactivity values in simulations of critical systems involving D2O. We discuss how the uncertainties in the thermal scattering cross sections of 2H(n,n)2H and 16O(n,n)16O propagate to the uncertainty of the calculated neutron multiplication factor, keff, in thermal critical assemblies with heavy water neutron moderator/reflector. The method of trial evaluated nuclear data files, in which specific cross sections are individually perturbed, is used to calculate the sensitivity coefficients of keff to the microscopic nuclear data, such as σs(E) characterized by σs,th. Large reactivity differences of up to ≃ 5-10 mk (500-1000 pcm) were observed using 2H and 16O data files with different elastic scattering data in MCNP5 simulations of the LANL HEU heavy-water solution thermal critical experiments included in the ICSBEP handbook.

  14. Interplay of the elastic and inelastic channels in the 16O+27Al scattering at Elab = 280 MeV

    NASA Astrophysics Data System (ADS)

    Cappuzzello, F.; Nicolosi, D.; Linares, R.; Oliveira, J. R. B.; Lubian, J.; Agodi, C.; Carbone, D.; Cavallaro, M.; de Faria, P. N.; Foti, A.; Rodrigues, M. R. D.

    2016-06-01

    Recent data indicated a nuclear rainbow-like pattern in the elastic scattering of 16O + 27Al at E_{lab}=100 MeV that arises from couplings of the ground to the low-lying states of the 27Al nucleus. Similar effect was identified in the elastic angular distribution of 16O + 12C at E_{lab}=281 and 330 MeV. These experiments show a crucial role of microscopic details of nuclear structure in the elastic scattering of heavy ions at energies well above the Coulomb barrier. In this work we investigate the 16O + 27Al system at E_{lab}=280 MeV for which a coupled channel calculation predicts a pronounced nuclear rainbow-like structure. Obtained experimental data show evidences of an important coupling of the elastic channel to the inelastic. Coupled channel calculations reproduce the experimental angular distributions when a re-normalization factor on the real part of the optical potential is introduced. A proper theoretical approach still requires a high degree of accuracy for the nuclear structure models and new tools to deal with collective excitations.

  15. Measurements and Modeling of 16O12C17O Spectroscopic Parameters at 2 μm

    NASA Astrophysics Data System (ADS)

    Jacquemart, David; Sung, Keeyoon; Brown, Linda; Coleman, Max; Mantz, Arlan; Smith, Mary Ann H.

    2014-06-01

    Nearly 1000 line intensities of 16O12C17O between 4604 and 5126 wn were measured using an isotopically-enriched mixture sample having 40 % (determined by mass spectrometry). Spectra were recorded at 0.0056 wn resolution with a Fourier transform spectrometer (Bruker IFS-125HR at JPL) configured to a Herriott cell with a 20.946 m absorption path. Since collisional narrowing effects were observed, the Rautian profile was systematically applied (instead of the Voigt profile) using a multispectrum retrieval procedure. Transition dipole moments and Herman-Wallis factors were derived for 15 bands, and a global comparison with theoretical calculations and predictions was obtained. Accuracies for the line intensities ranged between 2 - 3 % for strong bands and 6 - 30 % for weak bands. Retrieved line positions were calibrated using CO, HCl and some well-known 16O12C16O transitions. For both measured and calculated line positions, the accuracies fell between 0.1 - 1×10-3 wn. Self-broadening was also obtained for a few bands. Complete line lists were generated to support atmospheric remote sensing of the Earth (e.g., OCO-2 mission), Mars and Venus. Research described in this paper was performed at Connecticut College, the Jet Propulsion Laboratory, and California Institute of Technology, and NASA Langley Research Center, under contracts and cooperative agreements with the National Aeronautics and Space Administration.

  16. /sup 16/O(n, p)/sup 16/N: A fast neutron detector for rapid tissue inhomogeneity correction

    SciTech Connect

    Beach, J.L.; Watts, R.J.; Milavickas, L.R.

    1981-05-01

    We have devised a transit dose technique for fast neutron therapy treatment planning based on the /sup 16/O(n, p)/sup 16/N reaction in recirculating water, and have determined the effect of simulated bone and lung inhomogeneities in phantom. An effective threshold of 10.2 MeV in the /sup 16/O(n, p) reaction is exploited to detect transmitted neutrons without the need for detector collimation. This system has been demonstrated with 14 MeV (d, T) neutrons and with cyclotron produced p(42)+Be neutrons. /sup 16/N decays to the 6.13 MeV excited states of /sup 16/O in 7.14 s, allowing for easy identification by NaI(Tl) and for rapid recirculation. The transmission of fast neutrons can thus be related to an effective thickness of soft tissue, providing a rapid and direct measure of the effects of inhomogeneities under actual treatment conditions, with the 10 MeV threshold providing a useful degree of insensitivity to multiply scattered neutrons. Equivalent thicknesses of compact bone and lung relative to water were found to be 1.4 and 0.34 respectively, closely resembling the effective thicknesses for Cobalt-60 gamma rays.

  17. Including higher energy data in the R-matrix extrapolation of 12C(α , γ) 16O

    NASA Astrophysics Data System (ADS)

    Deboer, R.; Uberseder, E.; Azuma, R. E.; Best, A.; Brune, C.; Goerres, J.; Sayre, D.; Smith, K.; Wiescher, M.

    2015-10-01

    The phenomenological R-matrix technique has proved to be very successful in describing the cross sections of interest to nuclear astrophysics. One of the key reactions is 12C(α , γ) 16O, which has frequently been analyzed using R-matrix but usually over a limited energy range. This talk will present an analysis that, for the first time, extends above the proton and α1 separation energies taking advantage of a large amount of additional data. The analysis uses the new publicly released JINA R-matrix code AZURE2. The traditional reaction channels of 12C(α , γ) 16O, 12C(α ,α0) 12, and 16N(βα) 12C are included but are now accompanied by the higher energy reactions. By explicitly including higher energy levels, the uncertainty in the extrapolation of the cross section is significantly reduced. This is accomplished by more stringent constraints on interference combination and background poles by the additional higher energy data and by considering new information about subthresold states from transfer reactions. The result is the most comprehensive R-matrix analysis of the 12C(α , γ) 16O reaction to date. This research was supported in part by the ND CRC and funded by the NSF through Grant No. Phys-0758100, and JINA through Grant No. Phys-0822648.

  18. Geochemical and 3He/ 4He evidence for mantle and crustal contributions to geothermal fluids in the western Canadian continental margin

    NASA Astrophysics Data System (ADS)

    Clark, I. D.; Phillips, R. J.

    2000-12-01

    Isotopic and geochemical evidence together with helium isotopes are used to identify contributions of deep crustal to upper mantle volatile components in thermal waters at three sites across the western North American plate margin: (1) the low heat-flow forearc of the Cascadia subduction zone; (2) the high heat-flow volcanic arc; and (3) the interior crystalline terrain of the ancestral continental margin. Western continental margin hotsprings issue 50°C, low salinity Na-Cl water and N 2 gas with 0.25% CH 4. Stable isotopes and 14C indicate local meteoric recharge during the early Holocene. Redox is buffered by sulphate reduction, suggesting that the methane originates from a deeper source. The waters have high helium contents (He/He air=30) and a 3He-excess ( R/ Rair=0.27; 3He/ 3Heair=8), representing a mixture of radiogenic 4He production in crystalline rock with >10% He from subducted oceanic crust. Geophysical data indicate fluid-filled discontinuities in the subduction zone that may provide a pathway for He, and possibly for CH 4 and a saline fluid component from depth. In the Garibaldi belt of Quaternary arc-volcanism, 60°C Na-Cl hotsprings and 200°C geothermal well waters discharge from fractures in the basement rocks. δ18O and δ2H show the thermal waters to be a mixture of local recharge with up to 8% "andesitic" water from the upper mantle. He isotopes indicate a mantle origin ( R/ Rair=6.0), with a minor crustal signature, consistent with observations in the Cascadia range to the south and at other circum-Pacific volcanic arc settings. High PCO 2, an enriched δ13C DIC, elevated 3He/CO 2 ratios and elevated Cl - are likely to be derived from subducted Juan de Fuca plate sediments and pore waters. Thermal Na-SO 4 waters (up to 58°C) from the Omineca Crystalline Belt are locally recharged and have an unusually rapid circulation time of less than 40 years. This contrasts with their high radiogenic He content (176×10 -7 cc/g) with minimal mantle input

  19. Light microscopic autoradiographic localization of (/sup 3/H)pirenzepine and (/sup 3/H)(/sup -/)quinuclidinyl benzilate binding in human stellate ganglia

    SciTech Connect

    Yamamura, H.I.; Watson, M.; Wamsley, J.K.; Johnson, P.C.; Roeske, W.R.

    1984-08-13

    The LKB Ultrofilm method of autoradiography has been utilized to anatomically localize putative M/sub 1/ and M/sub 2/ muscarinic receptor subtypes in human stellate ganglia. Ten micron sections were labeled in vitro with either 1 nM of the classical antagonist (/sup 3/H)(/sup -/)quinuclidinyl benzilate ((/sup 3/H)(/sup -/)QNB) or 20 nM of the non-classical antagonist (/sup 3/H)pirenzepine ((/sup 3/H)PZ), using 1 ..mu..M atropine sulfate to define non-specific binding for both ligands. The results indicate that (/sup 3/H)(/sup -/)QNB and (/sup 3/H)PZ binding sites are distributed within the principal ganglion cells and nerve bundles.

  20. Phosphorus balance and mineral metabolism with 3 h daily hemodialysis.

    PubMed

    Ayus, J C; Achinger, S G; Mizani, M R; Chertow, G M; Furmaga, W; Lee, S; Rodriguez, F

    2007-02-01

    Poor control of mineral metabolism is independently associated with mortality in patients receiving hemodialysis. We analyzed data from a 12-month, prospective, non-randomized, controlled study of daily hemodialysis (DHD) (six sessions/week 3 h each) (n=26) vs conventional hemodialysis (CHD) (three sessions/week 4 h each) (n=51) for achievement of mineral metabolism goals and we performed a substudy of weekly dialytic phosphorus removal in DHD vs CHD. Phosphorus control was superior in the DHD group (% change from baseline to end-of-study -27+/-30% vs +7%+/-35% in the CHD group, P=0.0001). Percentage of patients using phosphate binders decreased from 77 to 40% among subjects on DHD, whereas these parameters did not change (76 vs 77%) in the CHD group (P=0.03 by Breslow-Day test for homogeneity of the odds ratios). Weekly mean phosphorus removal was higher in the DHD group (2452+/-720 mg/week vs 1572+/-366 mg/week, P=0.04). Mean normalized protein catabolic rate increased (0.90+/-0.43-1.22+/-0.26 g/kg/day, P=0.0013). DHD was also associated with an increase in the percent of subjects achieving three or more mineral metabolism goals (for phosphorus, calcium x phosphorus and parathyroid hormone) (15 vs 46%, P=0.046). In conclusion, DHD improves phosphorus control by increasing dialytic phosphorus removal while maintaining nutritional status and reducing the use of phosphate binders. The net effect allows for improved achievement of mineral metabolism goals. PMID:17191084

  1. Ethanol intake and sup 3 H-serotonin uptake II: A study in alcoholic patients using platelets sup 3 H-paroxetine binding

    SciTech Connect

    Daoust, M.; Boucly, P. ); Ernouf, D. ); Breton, P. ); Lhuintre, J.P.

    1991-01-01

    The kinetic parameters of {sup 3}H-paroxetine binding and {sup 3}H-serotonin uptake were studied in platelets of alcoholic patients. There was no difference between alcoholic and non alcoholic subjects in {sup 3}H-paroxetine binding. When binding and {sup 3}H-serotonin uptake were studied, in the same plasma of the same subjects, the Vmax of serotonin uptake was increased in alcoholics. The data confirm the involvement of serotonin uptake system in alcohol dependance and suggest that serotonin uptake and paroxetine binding sites may be regulated independently in this pathology.

  2. Binding of dexetimide and levetimide to [3H](+)pentazocine- and [3H]1,3-di(2-tolyl)guanidine-defined sigma recognition sites.

    PubMed

    DeHaven-Hudkins, D L; Hudkins, R L

    1991-01-01

    The potent antimuscarinic benzetimide and its resolved stereoisomers dexetimide and levetimide were tested for their affinities at sigma sites labelled by [3H](+)pentazocine or [3H]1,3-di(2-tolyl)guanidine. Levetimide was a potent and stereoselective inhibitor of [3H](+)pentazocine binding, with a Ki of 2.2 nM, while dexetimide was nine-fold less potent (Ki = 19 nM). Dexetimide and levetimide potently inhibited [3H]DTG binding although without stereoselectivity (Ki values of 65 and 103 nM, respectively). Levetimide may be a useful tool with which to investigate sigma recognition sites and sigma subtypes. PMID:1656155

  3. sigma opiates and certain antipsychotic drugs mutually inhibit (+)-(/sup 3/H)SKF 10,047 and (/sup 3/H)haloperidol binding in guinea pig brain membranes

    SciTech Connect

    Tam, S.W.; Cook, L.

    1984-09-01

    The relationship between binding of antipsychotic drugs and sigma psychotomimetic opiates to binding sites for the sigma agonist (+)-(/sup 3/H)SKF 10,047 (N-allylnormetazocine) and to dopamine D/sub 2/ sites was investigated. In guinea pig brain membranes, (+)-(/sup 3/H)SKF 10,047 bound to single class of sites with a K/sub d/ of 4 x 10/sup -8/ M and a B/sub max/ of 333 fmol/mg of protein. This binding was different from ..mu.., kappa, or delta opiate receptor binding. It was inhibited by opiates that produce psychotomimetic activities but not by opiates that lack such activities. Some antipsychotic drugs inhibited (+)-(/sup 3/H)SKF 10,047 binding with high to moderate affinities in the following order of potency: haloperidol > perphenazine > fluphenazine > acetophenazine > trifluoperazine > molindone greater than or equal to pimozide greater than or equal to thioridazine greater than or equal to chlorpromazine greater than or equal to triflupromazine. However, there were other antipsychotic drugs such as spiperone and clozapine that showed low affinity for the (+)-(/sup 3/H)SKF 10,047 binding sites. Affinities of antipsychotic drugs for (+)-(/sup 3/H)SKF 10,047 binding sites did not correlate with those for (/sup 3/H)spiperone (dopamine D/sub 2/) sites. (/sup 3/H)-Haloperidol binding in whole brain membranes was also inhibited by the sigma opiates pentazocine, cyclazocine, and (+)-(/sup 3/H)SKF 10,047. In the striatum, about half of the saturable (/sup 3/H)haloperidol binding was to (/sup 3/H)spiperone (D/sub 2/) sites and the other half was to sites similar to (+)-(/sup 3/H)SKF 10,047 binding sites. 15 references, 4 figures, 1 table.

  4. DNA Mismatch Repair Interacts with CAF-1- and ASF1A-H3-H4-dependent Histone (H3-H4)2 Tetramer Deposition.

    PubMed

    Rodriges Blanko, Elena; Kadyrova, Lyudmila Y; Kadyrov, Farid A

    2016-04-22

    DNA mismatch repair (MMR) is required for the maintenance of genome stability and protection of humans from several types of cancer. Human MMR occurs in the chromatin environment, but little is known about the interactions between MMR and the chromatin environment. Previous research has suggested that MMR coincides with replication-coupled assembly of the newly synthesized DNA into nucleosomes. The first step in replication-coupled nucleosome assembly is CAF-1-dependent histone (H3-H4)2 tetramer deposition, a process that involves ASF1A-H3-H4 complex. In this work we used reconstituted human systems to investigate interactions between MMR and CAF-1- and ASF1A-H3-H4-dependent histone (H3-H4)2 tetramer deposition. We have found that MutSα inhibits CAF-1- and ASF1A-H3-H4-dependent packaging of a DNA mismatch into a tetrasome. This finding supports the idea that MMR occurs before the DNA mismatch is packaged into the tetrasome. Our experiments have also revealed that CAF-1- and ASF1A-H3-H4-dependent deposition of the histone (H3-H4)2 tetramers does not interfere with MMR reactions. In addition, we have established that unnecessary degradation of the discontinuous strand that takes place in both DNA polymerase δ (Pol δ)- and DNA polymerase ϵ (Pol ϵ)-dependent MMR reactions is suppressed by CAF-1- and ASF1A-H3-H4-dependent deposition of the histone (H3-H4)2 tetramers. These data suggest that CAF-1- and ASF1A-H3-H4-dependent deposition of the histone (H3-H4)2 tetramers is compatible with MMR and protects the discontinuous daughter strand from unnecessary degradation by MMR machinery.

  5. Direct Total Cross Section Measurement of the 16O(α,γ)20Ne Reaction at Ec.m. = 2.26 MeV

    SciTech Connect

    Hager, Ulrike; Brown, James R.; Buchmann, Lothar R.; Carmona-Gallardo, Mariano; Erikson, Luke E.; Fallis, Jennifer S.; Greife, Uwe; Hutcheon, Dave; Ottewell, Dave; Ruiz, Chris; Sjue, Sky; Vockenhuber, Cristof

    2011-08-23

    In stellar helium burning, (16)O represents the endpoint of the helium-burning sequence due to the low rate of (16)O(alpha,gamma)(20)Ne. We present a new direct measurement of the total capture reaction rate of (16)O(alpha,gamma)(20)Ne at E(c.m.) = 2.26MeV employing the DRAGON recoil separator. For the first time, the total S factor and its contributing direct capture transitions could be determined in one experiment.

  6. Effect of hemoglobin on the uptake of /sup 3/H-norepinephrine and /sup 3/H-choline chloride into porcine cerebral arteries

    SciTech Connect

    Linnik, M.D.; Lee, T.J.F.

    1986-03-01

    Prolonged constriction of cerebral arteries often follows subarachnoid hemorrhage (SAH). SAH exposes hemoglobin (Hb) to cerebral arteries and Hb has been demonstrated to induce vasoconstriction as well as alter cerebrovascular neurogenic response characteristics. The effect of Hb on uptake of /sup 3/H-norepinephrine (/sup 3/H-NE) and /sup 3/H-choline chloride (/sup 3/H-ChCl) into porcine cerebral arteries was therefore examined. 0.5 to 50 ..mu..M porcine Hb caused a dose-dependent inhibition of /sup 3/H-NE uptake into the anterior (ANT), internal carotid (IC) and middle cerebral (MC) arteries of the pig. IC/sub 50/ values for uptake inhibition were: ANT, 31 ..mu..M; IC, 34 ..mu..M; MC, 37 ..mu..M. Porcine serum albumin (PSA) in the same concentration range also caused a decrease in /sup 3/H-NE uptake. An examination of protein-ligand interactions using column chromatography demonstrated binding of /sup 3/H-NE by both Hb and PSA. This protein binding may be responsible for part of the uptake inhibition. Hb and PSA had little effect on /sup 3/H-ChCl uptake into these arteries.

  7. Separation of carrier-free hafnium and lutetium radionuclides produced in 16O activated terbium metal target.

    PubMed

    Lahir, S; Banerjee, K; Nayak, D; Ramaswami, A; Das, N R

    2000-06-01

    Charged particle activation with approximately 88 MeV 16O7+ beam on natural terbium metal foil leads to the production of the short lived carrier-free radioisotopes 170,171Ta and their corresponding daughter products 170,171Hf and 170,171Lu in the target matrix. Liquid-liquid extraction with HDEHP diluted in cyclohexane was carried out for the separation of 170,171Hf and 170,171Lu from the bulk terbium in an aqueous HCl medium.

  8. {sup 16}O resonances near 4α threshold through {sup 12}C({sup 6}Li,d) reaction

    SciTech Connect

    Rodrigues, M. R. D.; Borello-Lewin, T.; Miyake, H.; Horodynski-Matsushigue, L. B.; Duarte, J. L. M.; Rodrigues, C. L.; Faria, P. Neto de; Cunsolo, A.; Cappuzzello, F.; Foti, A.; Agodi, C.; Cavallaro, M.; Napoli, M. di; Ukita, G. M.

    2014-11-11

    Several narrow alpha resonant {sup 16}O states were detected through the {sup 12}C({sup 6}Li,d) reaction, in the range of 13.5 to 17.5 MeV of excitation energy. The reaction was measured at a bombarding energy of 25.5 MeV employing the São Paulo Pelletron-Enge-Spectrograph facility and the nuclear emulsion technique. Experimental angular distributions associated with natural parity quasi-bound states around the 4α threshold are presented and compared to DWBA predictions. The upper limit for the resonance widths obtained is near the energy resolution (15 keV)

  9. Determination of astrophysical thermonuclear rates with a bubble chamber: The 12C(αγ)16O reaction case

    NASA Astrophysics Data System (ADS)

    DiGiovine, B.; Grames, J.; Henderson, D.; Holt, R. J.; Meekins, D.; Poelker, M.; Rehm, K. E.; Robinson, A.; Sonnenschein, A.; Suleiman, R.; Ugalde, C.

    2013-11-01

    The 12C(αγ)16O reaction rate is considered one of the most important unknown parameters in the physics of structure and evolution of massive stars. While extensive experimental campaigns have been performed trying to improve the quality of the measurements, the rate still holds very large uncertainties. Here we discuss a new experimantal scheme to measure the cross section of this reaction with a bubble chamber and a bremsstrahlung beam. The main advantage of the technique is a gain in the luminosity of several orders of magnitude when compared to other ongoing experiments.

  10. Excitation functions for production of heavy actinides from interactions of /sup 16/O with /sup 249/Cf

    SciTech Connect

    Chasteler, R.M.; Henderson, R.A.; Lee, D.; Gregorich, K.E.; Nurmia, M.J.; Welch, R.B.; Hoffman, D.C.

    1987-11-01

    Excitation functions have been measured for the production of isotopes of Bk through Fm in bombardments of /sup 249/Cf with 90- to 150-MeV /sup 16/O ions. A comparison of the maxima of the mass-yield curves measured in this experiment with those for the reactions of /sup 18/O ions with /sup 249/Cf shows different shifts from those that have been measured for reactions of the /sup 16,18/O and /sup 20,22/Ne ion pairs with /sup 248/Cm. However, the shifts appear similar to those recently measured for reactions of these ion pairs with /sup 254/Es.

  11. Detailed study and mean field interpretation of {sup 16}O+{sup 12}C elastic scattering at seven medium energies

    SciTech Connect

    Nicoli, M. P.; Haas, F.; Freeman, R. M.; Szilner, S.; Basrak, Z.; Morsad, A.; Satchler, G. R.; Brandan, M. E.

    2000-03-01

    Detailed measurements of the elastic scattering of {sup 16}O ions from {sup 12}C have been carried out at seven energies from 62 to 124 MeV, at center-of-mass angles from about 10 degree sign to about 145 degree sign . A coherent optical model analysis of these data has been performed using both the Woods-Saxon and the folding-model potentials. The extracted results are consistent with analyses of data at higher energies for this and similar light heavy-ion systems. Some model-independent spline forms for the real potentials were also investigated. (c) 2000 The American Physical Society.

  12. Assimilation of High 18O/16O Crust by Shergottite-Nakhlite-Chassigny (SNC) Magmas on Mars

    NASA Astrophysics Data System (ADS)

    Day, J. M.; Taylor, L. A.; Valley, J. W.; Spicuzza, M. J.

    2005-12-01

    There is significant geochemical evidence for assimilation of crustal material into sub-aerial, mantle-derived, terrestrial basaltic magmas. Some of the most powerful constraints on crustal assimilation come from oxygen isotope studies, because supracrustal rocks often have distinct 18O/16O ratios resulting from interaction with Earth's hydrosphere. From a planetary perspective, studies of carbonate concretions from meteorite ALH84001 have yielded evidence for low-temperature crustal interaction at or near the surface of its putative parent body, Mars. This finding raises the possibility that crustal assimilation processes may be tracked using oxygen isotopes in combination with geochemical data of other reputed martian (SNC) meteorites. The whole-rock oxygen isotope ratios (Laser fluorination δ18O = +4.21 to +5.85‰ VSMOW) of SNC meteorites, correlate with aspects of their incompatible element chemistry. Some of the oxygen isotope variability may be explained by post-magmatic alteration on Mars or Earth; however, it appears, based on petrographic and geochemical observations, that a number of SNC meteorites, especially Shergottites, retain the original whole-rock oxygen isotope values of their magmas prior to crystallisation. Correlations between oxygen isotopes and incompatible element geochemistry are consistent with assimilation of a high-18O/16O, incompatible-element rich, oxidizing crustal component by hot, mantle-derived magmas (δ18O = ~~4.2‰). A crustal component has previously been recognized from Sr-Nd-Os isotope systematics and oxygen fugacity measurements of SNC meteorites. Oxygen isotope evidence from SNC meteorites suggests high-18O/16O crustal contaminants on Mars result from low temperature (< 300°C) interaction with martian hydrosphere. The extent of apparent crustal contamination tracked by oxygen isotopes in SNC meteorites implies that the majority of martian crust may have undergone such interactions. Evidence for assimilation of

  13. The 18O/16O Ratio of 2-Billion-Year-Old Seawater Inferred from Ancient Oceanic Crust.

    PubMed

    Holmden, C; Muehlenbachs, K

    1993-03-19

    An oxygen isotope profile of the 2-billion-year-old Purtuniq ophiolite overlaps with similar profiles of younger ophiolites and the modern oceanic crust. This overlap implies (i) that there was a similar style of seawater-ocean crust interaction during the past 2 billion years; (ii) that the oxygen isotope composition of early Proterozoic seawater was similar to the modern value; (iii) that early Proterozoic sea-floor spreading rates were similar to, or greater than, average modern rates; and (iv) that early Proterozoic carbonate rocks and cherts with low (18)O/(16)O ratios do not reflect global-scale (18)O depletion of early Proterozoic oceans. PMID:17816892

  14. Nuclear rainbow in the 16O + 27AL system: The role of couplings at energies far above the barrier

    NASA Astrophysics Data System (ADS)

    Pereira, D.; Linares, R.; Oliveira, J. R. B.; Lubian, J.; Chamon, L. C.; Gomes, P. R. S.; Cunsolo, A.; Cappuzzello, F.; Cavallaro, M.; Carbone, D.; Foti, A.

    2012-04-01

    High precision elastic and inelastic angular distributions have been measured for the 16O + 27Al system at a beam energy of 100 MeV. The data analysis confirms a rainbow formation as already predicted by parameter-free Coupled Channel calculations. It also helps to reveal the crucial role of inelastic couplings in the rainbow formation for heavier systems even at energies far above the Coulomb barrier. This feature, well known in atomic/molecular scattering, is experimentally studied for the first time in Nuclear Physics.

  15. Rate constant measurement of the recombination reaction C[sub 3]H[sub 3] + C[sub 3]H[sub 3

    SciTech Connect

    Morter, C.L.; Farhat, S.K.; Adamson, J.D.; Glass, G.P.; Curl, R.F. )

    1994-07-14

    Using the technique of infrared kinetic absorption spectroscopy, the second-order rate constant for the recombination reaction of the propargyl radical (C[sub 3]H[sub 3] + C[sub 3]H[sub 3]) has been measured and found to have the value (1.2 [+-] 0.2) x 10[sup [minus]10] cm[sup 3] molecule[sup [minus]1] s[sup [minus]1] at 295 K. The radical was produced in a flow cell by excimer laser flash photolysis ([lambda] = 193 nm) of the precursors C[sub 3]H[sub 3]Cl or C[sub 3]H[sub 3]Br and detected using time-resolved IR absorption. Absolute concentrations of C[sub 3]H[sub 3] were determined by comparing the C[sub 3]H[sub 3] absorption intensity with that of the Br atom. This calibration scheme was checked by producing methyl radicals by photolysis of methyl bromide and comparing the rate constant for methyl recombination thus obtained with literature values. The quantum yield for HCl production from the photodissociation of C[sub 3]H[sub 3]Cl at 193 nm was determined to be 0.07 [+-] 0.01. 47 refs., 10 figs., 1 tab.

  16. Autoradiographic analysis of the in vivo distribution of 3H-imipramine and 3H-desipramine in brain: Comparison to in vitro binding patterns

    SciTech Connect

    Duncan, G.E.; Paul, I.A.; Fassberg, J.B.; Powell, K.R.; Stumpf, W.E.; Breese, G.R. )

    1991-03-01

    Using high resolution autoradiographic techniques, the distribution of radioactivity in forebrain and brainstem was assessed after 4 injection of 3H-impramine or 3H-desipramine. Results were compared with regional binding of the drugs to brain sections in vitro. Similar topographic binding of 3H-imipramine and 3H-desipramine was observed in vitro among brain regions, except in the paraventricular nucleus of the hypothalamus and locus coeruleus, where binding was greater for 3H-desipramine. For both 3H-desipramine and 3H-imipramine, some brain regions that exhibited high binding in vitro also showed high accumulation after in vivo injection. However, certain regions that contained high densities of binding sites for the antidepressant drugs as measured by in vitro binding showed very low accumulation of radioactivity after in vivo treatment. Such regions included the dentate gyrus of the hippocampus, layer 1 of piriform cortex, caudate-putamen, pontine and midbrain central gray, and cerebellar granular layer. Compared to in vitro binding of the drugs, the distribution of imipramine and desipramine in vivo appears more anatomically selective. For imipramine, primary sites of action in vivo, as indicated by the topographic distribution in brain, appear to be the locus coeruleus, hippocampus, lateral septal nucleus, and amygdala. For desipramine, the greatest accumulation in vivo was found in the locus coeruleus, paraventricular nucleus of the hypothalamus, and anterior thalamic nuclei.

  17. Nicotinic binding in rat brain: autoradiographic comparison of (/sup 3/H)acetylcholine, (/sup 3/H)nicotine, and (/sup 125/I)-alpha-bungarotoxin

    SciTech Connect

    Clarke, P.B.; Schwartz, R.D.; Paul, S.M.; Pert, C.B.; Pert, A.

    1985-05-01

    Three radioligands have been commonly used to label putative nicotinic cholinoceptors in the mammalian central nervous system: the agonists (/sup 3/H)nicotine and (/sup 3/H)acetylcholine ((/sup 3/H)ACh--in the presence of atropine to block muscarinic receptors), and the snake venom extract, (/sup 125/I)-alpha-bungarotoxin((/sup 125/I)BTX), which acts as a nicotinic antagonist at the neuromuscular junction. Binding studies employing brain homogenates indicate that the regional distributions of both (/sup 3/H)nicotine and (/sup 3/H)ACh differ from that of (/sup 125/I)BTX. The possible relationship between brain sites bound by (/sup 3/H)nicotine and (/sup 3/H)ACh has not been examined directly. The authors have used the technique of autoradiography to produce detailed maps of (/sup 3/H)nicotine, (/sup 3/H)ACh, and (/sup 125/I)BTX labeling; near-adjacent tissue sections were compared at many levels of the rat brain. The maps of high affinity agonist labeling are strikingly concordant, with highest densities in the interpeduncular nucleus, most thalamic nuclei, superior colliculus, medial habenula, presubiculum, cerebral cortex (layers I and III/IV), and the substantia nigra pars compacta/ventral tegmental area. The pattern of (/sup 125/I)BTX binding is strikingly different, the only notable overlap with agonist binding being the cerebral cortex (layer I) and superior colliculus. (/sup 125/I)BTX binding is also dense in the inferior colliculus, cerebral cortex (layer VI), hypothalamus, and hippocampus, but is virtually absent in thalamus. Various lines of evidence suggest that the high affinity agonist-binding sites in brain correspond to nicotinic cholinergic receptors similar to those found at autonomic ganglia; BTX-binding sites may also serve as receptors for nicotine and are possibly related to neuromuscular nicotinic cholinoceptors.

  18. Thermal neutron calibration of a tritium extraction facility using the /sup 6/Li(n,t)/sup 4/He//sup 197/Au(n,. gamma. )/sup 198/Au cross section ratio for standardization

    SciTech Connect

    Bretscher, M.M.; Smith, D.L.

    1980-08-01

    Absolute tritium activities in a neutron-activated metallic lithium samples have been measured by liquid scintillation methods to provide data needed for the determination of capture-to-fission ratios in fast breeder reactor spectra and for recent measurements of the /sup 7/Li(n,n't)/sup 4/He cross section. The tritium extraction facility used for all these experiments has now been calibrated by measuring the /sup 6/Li(n,t)/sup 4/He//sup 197/Au/n,..gamma..)/sup 198/Au activity ratio for thermal neutrons and comparing the result with the well-known cross sections. The calculated-to-measured activity ratio was found to be 1.033 +- 0.018. 2 figures, 20 tables.

  19. Quantitative Proteomic Analysis of Mouse Embryonic Fibroblasts and Induced Pluripotent Stem Cells Using 16O /18O labeling

    SciTech Connect

    Huang, Xin; Tian, Changhai; Liu, Miao; Wang, Yongxiang; Tolmachev, Aleksey V.; Sharma, Seema; Yu, Fang; Fu, Kai; Zheng, Jialin; Ding, Shi-Jian

    2012-04-06

    Induced pluripotent stem cells (iPSC) hold great promise for regenerative medicine as well as for investigations into the pathogenesis and treatment of various diseases. Understanding of key intracellular signaling pathways and protein targets that control development of iPSC from somatic cells is essential for designing new approaches to improve reprogramming efficiency. Here we report the development and application of an integrated quantitative proteomics platform for investigating differences in protein expressions between mouse embryonic fibroblasts (MEF) and MEF-derived iPSC. This platform consists of 16O/18O labeling, multidimensional peptide separation coupled with tandem mass spectrometry, and data analysis with UNiquant software. Using this platform a total of 2,481 proteins were identified and quantified from the 16O/18O-labeled MEF-iPSC proteome mixtures with a false discovery rate of 0.01. Among them, 218 proteins were significantly upregulated, while 247 proteins were significantly downregulated in iPSC compared to MEF. Many nuclear proteins, including Hdac1, Dnmt1, Pcna, Ccnd1, Smarcc1, and subunits in DNA replication and RNA polymerase II complex were found to be enhanced in iPSC. Protein network analysis revealed that Pcna functions as a hub orchestrating complicated mechanisms including DNA replication, epigenetic inheritance (Dnmt1) and chromatin remodeling (Smarcc1) to reprogram MEF and maintain stemness of iPSC.

  20. Charges and angular distributions of fast fragments produced in 3. 2-TeV /sup 16/O collisions with Pb

    SciTech Connect

    Gerbier, G.; Williams, W.T.; Price, P.B.; Guoxiao, R.; Vanderhaeghe, G.

    1987-11-30

    Out of 30 000 interactions of 3.2-TeV /sup 16/O nuclei in Pb, we found that no fast fragments had a charge Z>8, none with Zapprox. >5.5 had a charge that differed from an integer by as much as (1/3, and none with Zapprox. >5.5 had an angle to the beam >0.8 mrad. The cross section for production of a fast fragment with Z>8 or a stable particle with charge (19/3e, 20) / 3 e, (22/3e, or (23/3e is less than 240 ..mu..b at 90% confidence level. Using a measurement technique with a position resolution of 30 ..mu..rad, we found the transverse-momentum distributions for C, N, and O to be Gaussians with widths approx. =100 MeV/c, similar to those measured in projectile fragmentation of /sup 16/O at a factor 100 lower energy.

  1. The {sup 12}C({alpha}, {gamma}){sup 16}O E2 cross section at stellar energies

    SciTech Connect

    Descouvemont, P.; Dufour, M.

    2010-08-12

    The E2 component of the {sup 12}C({alpha}, {gamma}){sup 16}O cross section is investigated by a microscopic cluster model, and by R-matrix fits. The first approach provides S{sub E2}(300 keV){approx_equal}50 keV-b for ground-state transitions. In the R-matrix theory, we show that the background term plays a crucial role, and cannot be determined without ambiguity. Only an upper limit on the extrapolated S factor can be obtained [S{sub E2}(300 keV)<190 keV-b]. To constrain the R-matrix analysis, we use the GCM Asymptotic Normalization Constant (ANC) of the 2{sub 1}{sup +} level. This procedure strongly reduces the uncertainties on the R-matrix fit, and we end up with a recommended value of S{sub E2}(300 keV) =42{+-}2 keV-b. As ANC values derived from indirect methods are not consistent with the {sup 12}C({alpha}, {gamma}){sup 16}O cascade transitions to the 2{sub 1}{sup +} state, we suggest a remeasurement of this cross section.

  2. Human platelet dense granules: Improved isolation preliminary characterization of ( sup 3 H)-serotonin uptake and tetrabanazine-displaceable ( sup 3 H)-ketanserin binding

    SciTech Connect

    Chatterjee, D.; Anderson, G.M.; Chakraborty, M.; Cohen, D.J. )

    1990-01-01

    An improved method for the isolation of human platelet dense granules was developed. A good yield of highly enriched dense granules was obtained after mild sonication and Percoll gradient centrifugation. The method has facilitated characterization of the granule, permitting the first report of K{sub m} and V{sub max} values for ({sup 3}H)-serotonin uptake, as well as the first determination of K{sub d} and B{sub max} values for tetrabenazine-displaceable ({sup 3}H)-ketanserin binding, in the human platelet dense granule. The rates and affinities of ({sup 3}H)-serotonin uptake were similar to those previously reported for porcine dense granules. Tetrabenazine-displaceable ({sup 3}H)-ketanserin binding was observed with a K{sub d} similar to, and a B{sub max} approximately 10-fold lower than, that previously seen in bovine chromaffin granules.

  3. Synthesis ofN-(2-chloro-5-methylthiophenyl)-N'-(3-methyl-thiophenyl)-N'-[3H3]methylguanidine, l brace [3H3]CNS-5161 r brace

    SciTech Connect

    Gibbs, Andrew R.; Morimoto, Hiromi; VanBrocklin, Henry F.; Williams, Philip G.; Biegon, Anat

    2001-09-28

    The preparation of the title compound, [{sup 3}H{sub 3}]CNS-5161, was accomplished in three steps starting with the production of [{sup 3}H{sub 3}]iodomethane (CT{sub 3}I). The intermediate N-[{sup 3}H{sub 3}]methyl-3-(thiomethylphenyl)cyanamide was prepared in 77% yield by the addition of CT{sub 3}I to 3-(thiomethylphenyl)cyanamide, previously treated with sodium hydride. Reaction of this tritiated intermediate with 2-chloro-5-thiomethylaniline hydrochloride formed the guanidine compound [{sup 3}H{sub 3}]CNS-5161. Purification by HPLC gave the desired labeled product in an overall yield of 9% with greater than 96% radiochemical purity and a final specific activity of 66 Ci mmol{sup -1}.

  4. Binding of dexetimide and levetimide to ( sup 3 H)(+)pentazocine- and ( sup 3 H)1,3-Di(2-tolyl)guanidine-defined. sigma. recognition sites

    SciTech Connect

    Dehaven-Hudkins, D.L.; Hudkins, R.L. Virginia Commonwealth Univ., Richmond, VA )

    1991-01-01

    The potent antimuscarinic benzetimide and its resolved stereoisomers dexetimide and levetimide were tested for their affinities at {sigma} sites labelled by ({sup 3}H)(+)pentazocine or ({sup 3}H)1,3-di(2-tolyl)guanidine. Levetimide was a potent and stereoselective inhibitor of ({sup 3}H)(+)pentazocine binding, with a K{sub i} of 2.2 nM, while dexetimide was nine-fold less potent (K{sub i} = 19 nM). Dexetimide and levetimide potently inhibited ({sup 3}H)DTG binding although without stereoselectivity (K{sub i} values of 65 and 103 nM, respectively). Levetimide may be a useful tool with which to investigate {sigma} recognition sites and {sigma} subtypes.

  5. Incorporation of 3H from delta-(L-alpha-amino (4,5-3H)adipyl)-L-cysteinyl-D-(4,4-3H)valine into isopenicillin N.

    PubMed Central

    O'Sullivan, J; Bleaney, R C; Huddleston, J A; Abraham, E P

    1979-01-01

    1. delta-(L-alpha-Amino[4,5-3H]adipyl)-L-cysteinyl-D-[4,4-3H]valine has been synthesized from its constituent amino acids, the L-alpha-amino[4,5-3H]adipic acid being obtained by reduction with 3H2 of methyl 5-acetamido-5,5-diethoxycarbonylpent-2-enoate and subsequent decarboxylation and hydrolysis. 2. In a cell-free system prepared by lysis of protoplasts of Cephalosporium acremonium 3H was incorporated from the doubly labelled tripeptide into a compound that behaved like penicillin N or isopenicillin N. The relative specific radioactivities of the alpha-aminoadipyl and penicillamine moieties of the penicillin were the same (within experimental error) as those of the alpha-aminoadipic acid and valine residues respectively of the tripeptide. 3. The behaviour of the labelled alpha-aminoadipic acid from the penicillin to the L-amino acid oxidase of Crotalus adamanteus venom showed that it was mainly L-alpha-aminoadipic acid. 4. The results are consistent with the hypothesis that the carbon skeleton of the LLD-tripeptide is incorporated intact into the penicillin molecule and that the first product is isopenicillin N. PMID:575040

  6. Further study on fallout sup 3 H ingestion in Akita, Japan

    SciTech Connect

    Hisamatsu, S.; Takizawa, Y.; Katsumata, T.; Itoh, M.; Ueno, K.; Sakanoue, M. )

    1989-10-01

    To study fallout {sup 3}H ingestion in Japan, 16 separate food-group samples were collected from Akita City in northern Japan during early summer and late autumn in 1986. Furthermore, total diet samples which are duplicate composite food samples consumed by five or six persons for a period of 1 d were also obtained in Akita City. The {sup 3}H concentration in free water and that in a tissue-bound form were determined separately. Seasonal changes of {sup 3}H concentration in the food samples and the total diet samples were not found clearly. The average {sup 3}H concentration in the free water including tap water was 1.6 Bq L-1. The mean ratio of specific activity of tissue-bound {sup 3}H to that of {sup 3}H in free water was found to be 1.2. The average total {sup 3}H ingestion was estimated to be 4.0 Bq d-1, while the proportion of tissue-bound form {sup 3}H ingestion to total {sup 3}H ingestion was 11%. Cereal was the greatest contributing food group to ingestion of tissue-bound {sup 3}H. These findings were consistent with our previous results for food samples collected in 1985.

  7. Diffusivity fractionations of H2(16)O/H2(17)O and H2(16)O/H2(18)O in air and their implications for isotope hydrology.

    PubMed

    Barkan, Eugeni; Luz, Boaz

    2007-01-01

    We have determined the isotope effects of (17)O and (18)O substitution of (16)O in H(2)O on molecular diffusivities of water vapor in air by the use of evaporation experiments. The derived diffusion fractionation coefficients (17)alpha(diff) and (18)alpha(diff) are 1.0146 +/- 0.0002 and 1.0283 +/- 0.0003, respectively. We also determined, for the first time, the ratio ln((17)alpha(diff))/ln((18)alpha(diff)) as 0.5185 +/- 0.0002. This ratio, which is in excellent agreement with the theoretical value of 0.5184, is significantly smaller than the ratio in vapor-liquid equilibrium (0.529). We show how this new experimental information gives rise to (17)O excess in meteoric water, and how it can be applied in isotope hydrology.

  8. An isotopic-independent highly accurate potential energy surface for CO2 isotopologues and an initial (12)C(16)O2 infrared line list.

    PubMed

    Huang, Xinchuan; Schwenke, David W; Tashkun, Sergey A; Lee, Timothy J

    2012-03-28

    An isotopic-independent, highly accurate potential energy surface (PES) has been determined for CO(2) by refining a purely ab initio PES with selected, purely experimentally determined rovibrational energy levels. The purely ab initio PES is denoted Ames-0, while the refined PES is denoted Ames-1. Detailed tests are performed to demonstrate the spectroscopic accuracy of the Ames-1 PES. It is shown that Ames-1 yields σ(rms) (root-mean-squares error) = 0.0156 cm(-1) for 6873 J = 0-117 (12)C(16)O(2) experimental energy levels, even though less than 500 (12)C(16)O(2) energy levels were included in the refinement procedure. It is also demonstrated that, without any additional refinement, Ames-1 yields very good agreement for isotopologues. Specifically, for the (12)C(16)O(2) and (13)C(16)O(2) isotopologues, spectroscopic constants G(v) computed from Ames-1 are within ±0.01 and 0.02 cm(-1) of reliable experimentally derived values, while for the (16)O(12)C(18)O, (16)O(12)C(17)O, (16)O(13)C(18)O, (16)O(13)C(17)O, (12)C(18)O(2), (17)O(12)C(18)O, (12)C(17)O(2), (13)C(18)O(2), (13)C(17)O(2), (17)O(13)C(18)O, and (14)C(16)O(2) isotopologues, the differences are between ±0.10 and 0.15 cm(-1). To our knowledge, this is the first time a polyatomic PES has been refined using such high J values, and this has led to new challenges in the refinement procedure. An initial high quality, purely ab initio dipole moment surface (DMS) is constructed and used to generate a 296 K line list. For most bands, experimental IR intensities are well reproduced for (12)C(16)O(2) using Ames-1 and the DMS. For more than 80% of the bands, the experimental intensities are reproduced with σ(rms)(ΔI) < 20% or σ(rms)(ΔI∕δ(obs)) < 5. A few exceptions are analyzed and discussed. Directions for future improvements are discussed, though it is concluded that the current Ames-1 and the DMS should be useful in analyzing and assigning high-resolution laboratory or astronomical spectra. PMID:22462861

  9. Changes in [3H]-PK 11195 and [3H]-8-OH-DPAT binding following forebrain ischaemia in the gerbil.

    PubMed Central

    Kenny, B. A.; MacKinnon, A. C.; Spedding, M.; Brown, C. M.

    1993-01-01

    1. A high density of [3H]-PK 11195 binding sites was present in gerbil cortical membranes (Bmax [3H]-PK 11195 1360 +/- 71 fmol mg-1 protein) in comparison to rat cortical membranes (254 +/- 21 fmol mg-1 protein). This effect was species-specific as similar findings were obtained with hippocampal membranes (Bmax 1430 +/- 111 fmol mg-1 protein in gerbil, compared to 196 +/- 31 in rat). 2. RO 5-4864, also a peripheral type benzodiazepine compound, displayed low affinity for the [3H]-PK 11195 site in the gerbil (pKi 6.57 +/- 0.02 and 6.70 +/- 0.12 in hippocampus and cortex respectively) compared to rat (pKi 8.16 +/- 0.07 and 8.48 +/- 0.02). Central benzodiazepine compounds, diazepam and flunitrazepam, also displayed this trend. 3. RO 5-4864 displaced [3H]-PK 11195 binding from gerbil and rat cortical membranes through a competitive interaction with Hill slopes close to unity. In both tissues, saturation isotherms of [3H]-PK 11195 binding indicated that the presence of RO 5-4864 caused changes in Kd without any effect on Bmax. In kinetic experiments, the presence of RO 5-4864 failed to modify the rate of dissociation of [3H]-PK 11195 from equilibrium in both rat and gerbil cortical membranes.(ABSTRACT TRUNCATED AT 250 WORDS) PMID:8395288

  10. Radiogenic 3He/4He Estimates and Their Effect on Calculating Plio-Pleistocene Cosmogenic 3He Ages of Alluvial-Fan Terraces in the Lower Colorado River Basin, USA

    NASA Astrophysics Data System (ADS)

    Fenton, C.; Pelletier, J.

    2005-12-01

    Several alluvial-fan terraces near Topock, AZ were created by successive entrenchment of Pliocene and Pleistocene alluvial-fan gravels shed from the adjacent Black Mountains along the lower Colorado River corridor below Hoover Dam. These fans interfinger with and overlie main-stem Colorado River sands and gravels and grade to terrace levels that correspond with pre-existing elevations of the Colorado River. Absolute dates for the ages of Quaternary deposits on the lower Colorado River are rare and cosmogenic 3He age estimates of these surfaces would help constrain the timing of aggradation and incision in the lower Colorado River corridor. We analyzed individual basalt boulders from several terrace surfaces for total 3He/4He concentrations to calculate cosmogenic 3He ages of each fan terrace; 3He/4He values, expressed as R/Ra where Ra is the 3He/4He of air, range from 0.29 to 590. Black Mountain volcanic rocks have reported K-Ar ages between 15 and 30 Ma and basalt samples from adjacent alluvial fans contain 0.42 to 47× 1012 at/g of 4He, which has likely accumulated due to nuclear processes. The amount of radiogenic 3He/4He can be significant in old rocks with young exposure ages and can complicate determination of cosmogenic 3 He content. Alpha-decay of U, Th, and their daughter isotopes produces large amounts of 4He, whereas significant amounts of radiogenic 3He are only produced through the neutron bombardment of Li and subsequent beta-decay of tritium. We measured Li, U, Th, major and rare-earth element concentrations in whole-rock basalts and mineral separates. These concentrations are used to estimate the ratio of radiogenic helium contributed to the total helium system in our samples. Li concentrations typically range from 6 to 17 ppm, with one outlier of 62 ppm. U contents range from <0.1 to 2.7 ppm and Th contents range from 0.4 to 15.3 ppm. Based on these values, our calculations predict that the average radiogenic helium (R/Ra) contributed to the total

  11. Effects of α-cluster potentials for the O16+O16 fusion reaction and S factor

    NASA Astrophysics Data System (ADS)

    Kocak, G.; Karakoc, M.; Boztosun, I.; Balantekin, A. B.

    2010-02-01

    A joint analysis of the elastic-scattering angular distributions and fusion cross sections together with the S factor for the O16+O16 system near and below the Coulomb barrier is reported. To describe these observables within the framework of the optical model, a comparative study of microscopic α-α double-folding clusters and phenomenological shallow potentials with surface-transparent imaginary parts is performed. Although the phenomenological Woods-Saxon type of shallow real potentials is unable to provide a consistent explanation of these data, the α-α double-folding cluster potential obtained by considering the α-cluster structure of O16 provides a considerable improvement. The α-α double-folding cluster potential also reproduces the normalized resonant energy states of S32 for the N=24 cluster band.

  12. 18O/16O studies of fossil fissure fumaroles from the Valley of Ten Thousand Smokes, Alaska

    NASA Astrophysics Data System (ADS)

    Warner Holt, Elizabeth; Taylor, Hugh

    2001-03-01

    At three sample sites where there are good exposures of the upper 15 m of the 1912 ash-flow sheet in the Valley of Ten Thousand Smokes (VTTS), Alaska, 18O/16O studies indicate that fumarolic activity produced a very wide range of δ18O values (-0.1 to +12.6; n=32) in the groundmass adjacent to fossil fissure fumaroles. This contrasts sharply with the uniformity of δ18O in the groundmass away from fumarolic conduits (δ18O=+5.9 to +7.1; n=7) and in all of the feldspar phenocrysts (δ18O=+6.11 to +7.51 for 11 samples from this study and Hildreth 1987), independent of whether these were collected from fossil fumaroles or from unaltered tuff. Only one sample contained feldspars that were even slightly 18O-enriched relative to the others (cloudy plagioclase δ18O=+8.45), and this sample also contained the most 18O-enriched groundmass of any of those analyzed (δ18O=+12.6). This preservation of primary magmatic δ18O values in the VTTS feldspar phenocrysts is clearly a consequence of the extremely short time span (i.e., 1912 to 1923) of vigorous, high-temperature, fumarolic activity in the 1912 ash-flow sheet. These 18O/16O systematics are strikingly similar to those discovered in the 2.8-Ma intracaldera Chegem Tuff (Gazis et al. 1996) and in the fossil fumaroles in the outflow sheet of the 0.76 Ma Bishop Tuff (Holt and Taylor 1998), thus confirming that a similar type of fumarolic meteoric-hydrothermal activity occurred above the zone of intense welding in all three of these ash-flow tuffs. This is particularly important, because it provides a direct linkage between the older tuffs and the actual observations at the VTTS of steam chemistry, water/rock interaction, circulation geometry, flow velocities, and fumarolic temperatures (up to 645°C). The 18O/16O effects in the VTTS can all be explained in terms of a two-stage history: (a) an early, 10- to 15-year-long, high-temperature (>450°C), fumarolic 18O-depletion event (groundmass δ18O=-0.1 to +4.8); and (b) a

  13. Photochemical fractionation of 16O in the space medium modeled by resonance excitation of CO by H-Lyman alpha.

    PubMed

    Arrhenius, G; Corrigan, M J; Fitzgerald, R W

    1988-01-01

    Inferences about the formation of primordial matter in our solar system rest on analysis of the earliest preserved materials in meteorites, of the structure of the solar system today, and of matter in evolving stellar systems elsewhere. The isotope distribution in meteorites suggests that molecular excitation processes similar to those observed today in circumstellar regions and dark interstellar clouds were operating in the early solar nebula. Laboratory model experiments together with these observations give evidence on the thermal state of the source medium from which refractory meteoritic dust formed. They indicate that resonance excitation of the broad isotopic bands of molecules such as 12C16O, MgO, O2, AlO, and OH by strong UV line sources such as H-L alpha, Mg II, H beta, and Ca II may induce selective reactions resulting in the anomalous isotopic composition of oxygen and possibly other elements in refractory oxide condensates in meteorites.

  14. Adiabatic and coupled channels calculations for near barrier fusion of 16O +238U using realistic nucleon-nucleon interaction

    NASA Astrophysics Data System (ADS)

    Ismail, M.; Seif, W. M.; Botros, M. M.

    2016-04-01

    We investigate the fusion cross-section and the fusion barrier distribution of 16O +238U at near- and sub-barrier energies. We use an interaction potential generated by the semi-microscopic double folding model-based on density dependent (DD) form of the realistic Michigan-three-Yukawa (M3Y) Reid nucleon-nucleon (NN) interaction. We studied the role of both the static and dynamic deformations of the target nucleus on the fusion process. Rotational and vibrational degrees of freedom of 238U-nucleus are considered. We found that the deformation and the octupole vibrations in 238U enhance its sub-barrier fusion cross-section. The signature of the the octupole vibrational modes of 238U appears clearly in its fusion barrier distribution profile.

  15. CO2 pressure broadening and shift coefficients for the 2-0 band of 12C16O

    NASA Astrophysics Data System (ADS)

    Hashemi, R.; Predoi-Cross, A.; Dudaryonok, A. S.; Lavrentieva, N. N.; Vandaele, A. C.; Vander Auwera, J.

    2016-08-01

    Fourier transform absorption spectra of the 2-0 band of 12C16O mixed with CO2 have been recorded at total pressures from 156 to 1212 hPa and at 4 different temperatures between 240 K and 283 K. CO2 pressure-induced line broadening and line shift coefficients, and the temperature dependence of the former have been measured including line mixing using a multi-spectrum non-linear least squares fitting technique. Different line shape models have been considered to take into account the Dicke narrowing or speed dependence effects. Measured line-shape parameters were compared with theoretical values, calculated for individual temperatures using a semi-empirical method and the Exponential Power Gap (EPG) law.

  16. The Rovibrational Intensities of Five Absorption Bands of (12)C(16)O2 Between 5218 and 5349/cm

    NASA Technical Reports Server (NTRS)

    Giver, Lawrence P.; Brown, Linda R.; Chackerian, Charles, Jr.; Freedman, Richard S.; Gore, Warren J. (Technical Monitor)

    2002-01-01

    Absolute line intensities, band intensities, and Herman-Wallis parameters were measured for the (01(sup 1)2)(sub I) from (00(sup 0)0)(sub I) perpendicular band of (12)C(16)O2 centered at 5315/cm, along with the three nearby associated hot bands: (10(sup 0)2)(sub II) from (01(sup 1)0)(sub I) at 5248/cm, (02(sup 2))(sub I) from (01(sup 1)0)(sub I) at 5291/cm, and (10(sup 0)2)(sub I) from (01(sup 1)0)(sub I) at 5349/cm. The nearby parallel hot band (30(sup 0))(sub I) from (10(sup 0)0)(sub II) at 5218/cm was also included in this study.

  17. Statistical Model to Analyze Quantitative Proteomics Data Obtained by 18O/16O Labeling and Linear Ion Trap Mass Spectrometry

    PubMed Central

    Jorge, Inmaculada; Navarro, Pedro; Martínez-Acedo, Pablo; Núñez, Estefanía; Serrano, Horacio; Alfranca, Arántzazu; Redondo, Juan Miguel; Vázquez, Jesús

    2009-01-01

    Statistical models for the analysis of protein expression changes by stable isotope labeling are still poorly developed, particularly for data obtained by 16O/18O labeling. Besides large scale test experiments to validate the null hypothesis are lacking. Although the study of mechanisms underlying biological actions promoted by vascular endothelial growth factor (VEGF) on endothelial cells is of considerable interest, quantitative proteomics studies on this subject are scarce and have been performed after exposing cells to the factor for long periods of time. In this work we present the largest quantitative proteomics study to date on the short term effects of VEGF on human umbilical vein endothelial cells by 18O/16O labeling. Current statistical models based on normality and variance homogeneity were found unsuitable to describe the null hypothesis in a large scale test experiment performed on these cells, producing false expression changes. A random effects model was developed including four different sources of variance at the spectrum-fitting, scan, peptide, and protein levels. With the new model the number of outliers at scan and peptide levels was negligible in three large scale experiments, and only one false protein expression change was observed in the test experiment among more than 1000 proteins. The new model allowed the detection of significant protein expression changes upon VEGF stimulation for 4 and 8 h. The consistency of the changes observed at 4 h was confirmed by a replica at a smaller scale and further validated by Western blot analysis of some proteins. Most of the observed changes have not been described previously and are consistent with a pattern of protein expression that dynamically changes over time following the evolution of the angiogenic response. With this statistical model the 18O labeling approach emerges as a very promising and robust alternative to perform quantitative proteomics studies at a depth of several thousand proteins

  18. Neotropical eocene coastal floras and [sup 18]O/[sup 16]O-estimated warmer vs. cooler equatorial waters

    SciTech Connect

    Graham, A. )

    1994-03-01

    The history of the earth's sea-surface temperature (SST) in equatorial regions during the Tertiary is unsettled because of uncertainty as to the presence and extent of glaciers during the Paleogene. The [sup 16]O trapped in glaciers and subsequently released back to the ocean basins as meltwater during interglacials affects the [sup 18]O/[sup 16]O ratio of sea water, one of the variables that must be known for oxygen isotope paleotemperature analysis of calcareous fossils. Estimates of SST range from [approximately]18 to 20 C, assuming an ice-free earth, to [approximately]28 C assuming glaciers were present in the Paleogene. Low latitude SST presently averages 28C, so the former estimate gives a value 8 to 10 C cooler than present, while the latter gives a value as warm or slightly warmer than present. The figures are important for interpreting terrestrial vegetational history because the temperature differential between low and high latitudes is a major factor in determining global climates through the control of poleward transfer of heat. The middle( ) to late Eocene Gatuncillo Formation palynoflora of Panama was deposited at the ocean-continental interface at [approximately]9[degrees]N latitude. The individual components and paleocommunities are distinctly tropical and similar to the present vegetation along the Atlantic coast of southern Central America. This is consistent with data emerging from other recently studied tropical coastal biotas and represents a contribution from paleobiology toward eventually resolving the problem of Eocene equatorial marine environments. Collectively, the evidence is beginning to favor a model of Eocene SST near present values. 50 refs., 1 fig., 2 tabs.

  19. ( 3 H)lysergic acid diethylamide: cellular autoradiographic localization in rat brain.

    PubMed

    Diab, I M; Freedman, D X; Roth, L J

    1971-09-10

    Intravenous administration of [(3)H]lysergic acid diethylamide(LSD) to rats resulted in accumulation of the drug in the brain within 15 minutes. Autoradiographic methods were used to differentiate free and bound [(3)H]LSD in brain tissue. Free [(3)H]LSD was generally distributed in the pituitary and pineal glands, cerebellum, hippocampus,and choroid plexus. Bound [(3)H]LSD was localized in neurons of the cortex, caudate nucleus, midbrain, and medulla,as well as in choroid plexus epithelium.

  20. [3H]benzo[a]pyrene utilization in rats following tracheal implant exposure.

    PubMed

    Marchok, A C; Fleming, G S; Tomkins, B A; Griest, W H

    1989-05-31

    Open-ended rat tracheal implants (OETI) were exposed to 40 micrograms [3H]benzo[a]pyrene (B[a]P)-gelatin pellets and the 3H activity in the OETI, the host's tissues and excretia was determined 3-96 h after insertion of the pellets. The radioactivity in the OETI reached near peak activity by 3 h, and decreased almost 10-fold by 24 h. Most of the activity was associated with parent B[a]P throughout the 95 h. The 3H activity in the surrounding tissue also was mostly associated with B[a]P, but the 3H activity in the liver, kidney, blood and urine was mostly associated with water-soluble plus conjugated metabolites. In the feces, 68% of the 3H activity was in B[a]P at 3 h, but mostly organic as well as water-soluble plus conjugated metabolites were extracted from it throughout the remaining 96 h. Forty-eight hours after insertion of the B[a]P pellets, the feces contained almost 16% of the total 3H activity. Pre-exposure of the OETI to B[a]P for 4 days before insertion of the [3H]B[a]P pellets stimulated metabolism of B[a]P in the tracheas approximately 2-fold, but had no significant effect on the host tissues. PMID:2728007