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Sample records for 6li 7li nuclear

  1. Transport properties derived from ion-atom collisions: 6Li-6Li+ and 6Li-7Li+ Cases

    NASA Astrophysics Data System (ADS)

    Bouledroua, Moncef; Bouchelaghem, Fouzia; LPR Team

    2014-10-01

    This investigation treats quantum-mechanically the ion- atom collisions and computes the transport coefficients, such as the coefficients of mobility and diffusion. For the case of lithium, the calculations start by determining the gerade and ungerade potential curves through which ionic lithium approaches ground lithium. Then, by considering the isotopic effects and nuclear spins, the elastic and charge-transfer cross sections are calculated for the case of 6Li+and7Li+ colliding with 6Li. Finally, the temperature-dependent diffusion and mobility coefficients are analyzed, and the results are contrasted with those obtained from literature. The main results of this work have been recently published in. This work has been realized within the frames of the CNEPRU Project D01120110036 of the Algerian Ministry of Higher Education.

  2. Gamow shell model description of radiative capture reactions 6Li(p, γ)7Be and 6Li(n, γ)7Li

    NASA Astrophysics Data System (ADS)

    Dong, G. X.; Michel, N.; Fossez, K.; Płoszajczak, M.; Jaganathen, Y.; Betan, R. M. Id

    2017-04-01

    Background. According to standard stellar evolution, lithium abundance is believed to be a useful indicator of the stellar age. However, many evolved stars like red giants show huge fluctuations around expected theoretical abundances that are not yet fully understood. The better knowledge of nuclear reactions that contribute to the creation and destruction of lithium can help to solve this puzzle. Purpose. In this work we apply the Gamow shell model formulated in the coupled-channel representation to investigate the mirror radiative capture reactions 6Li(p, γ)7Be and 6Li(n, γ)7Li. Method. The cross-sections are calculated using a translationally invariant Hamiltonian with the finite-range interaction which is adjusted to reproduce spectra, binding energies and one-nucleon separation energies in 6–7Li, 7Be. The reaction channels are built by coupling the wave functions of ground state {1}1+ and excited states {3}1+, {0}1+, {2}1+ of 6Li with the projectile wave function in different partial waves. Results. We include all relevant E1, M1, and E2 transitions from the initial continuum states to the final bound states J=3/{2}1- and J=1/{2}- of 7Li and 7Be. Our microscopic astrophysical factor for the 6Li(p, γ)7Be reaction follows the average trend of the experimental value as a function of the center of mass energy. For {}6{Li}(n,γ ){}7{Li}, the calculated cross section agrees well with the data from the direct measurement of this reaction at stellar energies. Conclusion. We demonstrate that the s-wave radiative capture of proton (neutron) to the first excited state {J}π =1/{2}1+ of 7Be (7Li) is crucial and increases the total astrophysical S-factor by about 40%.

  3. Lamb shifts and hyperfine structure in 6Li+ and 7Li+: Theory and experiment

    NASA Astrophysics Data System (ADS)

    Riis, E.; Sinclair, A. G.; Poulsen, O.; Drake, G. W. F.; Rowley, W. R. C.; Levick, A. P.

    1994-01-01

    High-precision laser-resonance measurements accurate to +/-0.5 MHz or better are reported for transitions among the 1s2s 3S1-1s2p 3PJ hyperfine manifolds for each of J=0, 1, and 2 in both 6Li+ and 7Li+. A detailed analysis of hyperfine structure is performed for both the S and P states, using newly calculated values for the magnetic dipole and electric quadrupole coupling constants, and the hyperfine shifts subtracted from the measurements. The resulting transition frequencies are then analyzed on three different levels. First, the isotope shifts in the fine-structure splittings are calculated from the relativistic reduced mass and recoil terms in the Breit interaction, and compared with experiment at the +/-0.5-MHz level of accuracy. This comparison is particularly significant because J-independent theoretical uncertainties reduce through cancellation to the +/-0.01-MHz level. Second, the isotope shifts in the full transition frequencies are used to deduce the difference in rms nuclear radii. The result is Rrms(6Li)-Rrms(7Li)=0.15+/-0.01 fm, in agreement with nuclear scattering data, but with substantially improved accuracy. Third, high-precision calculations of the low-order non-QED contributions to the transition frequencies are subtracted from the measurements to obtain the residual QED shifts. The isotope-averaged and spin-averaged effective shift for 7Li+ is 37 429.40+/-0.39 MHz, with an additional uncertainty of +/-1.5 MHz due to finite nuclear size corrections. The accuracy of 11 parts per million is the best two-electron Lamb shift measurement in the literature, and is comparable to the accuracies achieved in hydrogen. Theoretical contributions to the two-electron Lamb shift are discussed, including terms of order (αZ)4 recently obtained by Chen, Cheng, and Johnson [Phys. Rev. A 47, 3692 (1993)], and the results used to extract a QED shift for the 2 3S1 state. The result of 30 254+/-12 MHz is shown to be in good accord with theory (30 250+/-30 MHz) when

  4. Line shift, line asymmetry, and the ^6Li/^7Li isotopic ratio determination

    NASA Astrophysics Data System (ADS)

    Cayrel, R.; Steffen, M.; Chand, H.; Bonifacio, P.; Spite, M.; Spite, F.; Petitjean, P.; Ludwig, H.-G.; Caffau, E.

    2007-10-01

    Context: Line asymmetries are generated by convective Doppler shifts in stellar atmospheres, especially in metal-poor stars, where convective motions penetrate to higher atmospheric levels. Such asymmetries are usually neglected in abundance analyses. The determination of the ^6Li/^7Li isotopic ratio is prone to suffering from such asymmetries, as the contribution of ^6Li is a slight blending reinforcement of the red wing of each component of the corresponding ^7Li line, with respect to its blue wing. Aims: The present paper studies the halo star HD 74000 and estimates the impact of convection-related asymmetries on the Li isotopic ratio determination. Methods: Two methods are used to meet this aim. The first, which is purely empirical, consists in deriving a template profile from another element that can be assumed to originate in the same stellar atmospheric layers as Li I, producing absorption lines of approximately the same equivalent width as individual components of the ^7Li I resonance line. The second method consists in conducting the abundance analysis based on NLTE line formation in a 3D hydrodynamical model atmosphere, taking into account the effects of photospheric convection. Results: The results of the first method show that the convective asymmetry generates an excess absorption in the red wing of the ^7Li absorption feature that mimics the presence of ^6Li at a level comparable to the hitherto published values. This opens the possibility that only an upper limit on ^6Li/^7Li has thus far been derived. The second method confirms these findings. Conclusions: From this work, it appears that a systematic reappraisal of former determinations of ^6Li abundances in halo stars is warranted. Based on observations carried out at the European Southern Observatory (ESO), under prog. ID 75.D-0600. Tables 1-3, and additional references are only available in electronic form at http://www.aanda.org

  5. Theory of laser enhancement and suppression of cold reactions: the fermion-boson 6Li+7Li2<-->(variant Planck's over 2pi omega0) 6Li7Li+7Li radiative collision.

    PubMed

    Li, Xuan; Parker, Gregory A; Brumer, Paul; Thanopulos, Ioannis; Shapiro, Moshe

    2008-03-28

    We present a nonperturbative time-dependent quantum mechanical theory of the laser catalysis and control of a bifurcating A+BC<-->(variant Planck's over 2pi omega(0))ABC*(v)<-->(variant Planck's over 2pi omega(0) )AB+C reaction, with ABC*(v) denoting an intermediate, electronically excited, complex of ABC in the vth vibrational state. We apply this theory to the low collision energy fermion-boson light-induced exchange reaction, (6)Li((2)S)+(7)Li(2)((3)Sigma(u)(+))<-->(variant Planck's over 2pi omega(0))((6)Li(7)Li(7)Li)*<-->(variant Planck's over 2pi omega(0))(6)Li(7)Li((3)Sigma(+))+(7)Li((2)S). We show that at very low collision energies and energetically narrow (approximately 0.01 cm(-1)) initial reactant wave packets, it is possible to tune the yield of the exchange reaction from 0 to near-unity (yield >or=99%) values. Controllability is somewhat reduced at collisions involving energetically wider (approximately 1 cm(-1)) initial reactant wave packets. At these energetic bandwidths, the radiative reactive control, although still impressive, is limited to the 0%-76% reactive-probabilities range.

  6. Polarization potentials for the 208Pb(7Li,6Li)209Pb transfer

    NASA Astrophysics Data System (ADS)

    Keeley, N.; Rusek, K.

    1997-12-01

    Recent optical model analyses of near-barrier 7Li+208Pb elastic scattering data found a peak in the energy dependence of WOM, the strength of the imaginary part of the optical model potential at the strong absorption radius. It was speculated that this might be due to the polarization potentials produced by couplings to the 208Pb(7Li,6Li)209Pb transfer channels. In this Brief Report we show explicitly that such couplings do indeed produce polarization potentials with the same energy dependence as that observed for the empirical optical potentials.

  7. Fast neutron measurements with 7Li and 6Li enriched CLYC scintillators

    NASA Astrophysics Data System (ADS)

    Giaz, A.; Blasi, N.; Boiano, C.; Brambilla, S.; Camera, F.; Cattadori, C.; Ceruti, S.; Gramegna, F.; Marchi, T.; Mattei, I.; Mentana, A.; Million, B.; Pellegri, L.; Rebai, M.; Riboldi, S.; Salamida, F.; Tardocchi, M.

    2016-07-01

    The recently developed Cs2LiYCl6:Ce (CLYC) crystals are interesting scintillation detectors not only for their gamma energy resolution (<5% at 662 keV) but also for their capability to identify and measure the energy of both gamma rays and fast/thermal neutrons. The thermal neutrons were detected by the 6Li(n,α)t reaction while for the fast neutrons the 35Cl(n,p)35S and 35Cl(n,α)32P neutron-capture reactions were exploited. The energy of the outgoing proton or α particle scales linearly with the incident neutron energy. The kinetic energy of the fast neutrons can be measured using both the Time Of Flight (TOF) technique and using the CLYC energy signal. In this work, the response to monochromatic fast neutrons (1.9-3.8 MeV) of two CLYC 1″×1″ crystals was measured using both the TOF and the energy signal. The observables were combined to identify fast neutrons, to subtract the thermal neutron background and to identify different fast neutron-capture reactions on 35Cl, in other words to understand if the detected particle is an α or a proton. We performed a dedicated measurement at the CN accelerator facility of the INFN Legnaro National Laboratories (Italy), where the fast neutrons were produced by impinging a proton beam (4.5, 5.0 and 5.5 MeV) on a 7LiF target. We tested a CLYC detector 6Li-enriched at about 95%, which is ideal for thermal neutron measurements, in parallel with another CLYC detector 7Li-enriched at more than 99%, which is suitable for fast neutron measurements.

  8. Asymptotic and near-target direct breakup of 6Li and 7Li

    NASA Astrophysics Data System (ADS)

    Kalkal, Sunil; Simpson, E. C.; Luong, D. H.; Cook, K. J.; Dasgupta, M.; Hinde, D. J.; Carter, I. P.; Jeung, D. Y.; Mohanto, G.; Palshetkar, C. S.; Prasad, E.; Rafferty, D. C.; Simenel, C.; Vo-Phuoc, K.; Williams, E.; Gasques, L. R.; Gomes, P. R. S.; Linares, R.

    2016-04-01

    Background: Li,76 and 9Be are weakly bound against breakup into their cluster constituents. Breakup location is important for determining the role of breakup in above-barrier complete fusion suppression. Recent works have pointed out that experimental observables can be used to separate near-target and asymptotic breakup. Purpose: Our purpose is to distinguish near-target and asymptotic direct breakup of Li,76 in reactions with nuclei in different mass regions. Method: Charged particle coincidence measurements are carried out with pulsed Li,76 beams on 58Ni and 64Zn targets at sub-barrier energies and compared with previous measurements using 208Pb and 209Bi targets. A detector array providing a large angular coverage is used, along with time-of-flight information to give definitive particle identification of the direct breakup fragments. Results: In interactions of 6Li with 58Ni and 64Zn, direct breakup occurs only asymptotically far away from the target. However, in interactions with 208Pb and 209Bi, near-target breakup occurs in addition to asymptotic breakup. Direct breakup of 7Li into α -t is not observed in interactions with 58Ni and 64Zn. However, near-target dominated direct breakup was observed in measurements with 208Pb and 209Bi. A modified version of the Monte Carlo classical trajectory model code platypus, which explicitly takes into account lifetimes associated with unbound states, is used to simulate sub-barrier breakup reactions. Conclusions: Near-target breakup in interactions with Li,76 is an important mechanism only for the heavy targets 208Pb and 209Bi. There is insignificant near-target direct breakup of 6Li and no direct breakup of 7Li in reactions with 58Ni and 64Zn. Therefore, direct breakup is unlikely to suppress the above-barrier fusion cross section in reactions of Li,76 with 58Ni and 64Zn nuclei.

  9. Study of the /sup 7/Li(/sup 3/He,. cap alpha. )/sup 6/Li* reaction

    SciTech Connect

    Lin, B.S.C.

    1980-01-01

    Differential cross sections for formation of the 5.37 MeV (J'' = 2/sup +/, T = 1) level in /sup 6/Li have been measured via the reaction /sup 7/Li(/sup 3/He,..cap alpha..)/sup 6/Li at incident /sup 3/He energies in the range 0.7 to 2.5 MeV and for angles in the range 20/sup 0/ less than or equal to theta (Lab) less than or equal to 160/sup 0/. Data for the g.s., 2.18 and 3.56 MeV excited states of /sup 6/Li were also obtained. The results for the g.s. and the first two excited states are in good agreement with previous measurements and show no clear resonance structure. The excitation function for the 5.37 MeV state, however, exhibits resonance structure at incident /sup 3/He energies of 1.45 and 2.15 MeV corresponding to formation of states in the compound nucleus, /sup 10/B, at 18.8 and 19.3 MeV excitation respectively. The experimental data were compared with the results of DWBA calculations using the computer code DWUCK4. Coincident events between the first emitted alpha particle and the decay alpha's or proton's were detected using a counter telescope in the reaction plane at several appropriately chosen angle pairs at an incident /sup 3/He energy of 2.15 MeV. Branching ratios for the allowed decay modes /sup 5/He + p and ..cap alpha.. + p + n, as well as the isospin forbidden decay into ..cap alpha.. + d, were deduced from the data.

  10. An atomic beam of 6Li7Li for high resolution spectroscopy from matrix isolation sublimation

    NASA Astrophysics Data System (ADS)

    Oliveira, A. N.; Sacramento, R. L.; Silva, B. A.; Uhlmann, F. O.; Wolff, W.; Cesar, C. L.

    2016-07-01

    We propose the Matrix Isolation Sublimation (MlSu) technique for generating cold lithium atoms for the measurement of the 6Li - 7Li isotope shift in D1 and D2 transitions. The technique is capable of generating cold 6Li and 7Li beams at 4 K with forward velocity of 125 m/s. Using this beam we offer a distinguished source of lithium atoms for transitions measurements, adding a new possibility to make high resolution spectroscopy towards improving the experimental checks of the theory.

  11. Reactions induced by 18 MeV 6He beam on 6Li, 7Li and 12C

    NASA Astrophysics Data System (ADS)

    Milin, M.; Cherubini, S.; Davinson, T.; Di Pietro, A.; Figuera, P.; Miljanić, Đ.; Musumarra, A.; Ninane, A.; Ostrowski, A. N.; Pellegriti, M. G.; Shotter, A. C.; Soić, N.; Spitaleri, C.; Zadro, M.

    2004-12-01

    The 6He+ 6,7Li and 6He+ 12C scattering and reactions have been studied using a 18 MeV 6He beam. Experimental results for the elastic scattering on all three targets are in fair agreement with optical model predictions, using the potentials found in the analysis of the 6Li scattering on the same targets and at close energies. Large cross sections are observed for α-transfer reactions to some states of 10Be. The sequential decay reactions 6He+ 6Li→ 6He+ α+ d, 6He+ 6Li→2 α+ t+ n, 6He+ 7Li→ 6He+ α+ t and 6He+ 12C→ 10Be+2 α were clearly seen and analysing them α-clustering of some states in 6Li, 7Li, 8Be, 9Be, 10Be and 14C was recognized.

  12. Progress towards a test of the universality of free fall using a 6Li/7Li atom interferometer

    NASA Astrophysics Data System (ADS)

    Kim, Geena; Hamilton, Paul; Schlippert, Dennis; Müller, Holger

    2011-05-01

    Many extensions of the standard model of physics, e.g. Kaluza-Klein theories, string theory, and supersymmetry, introduce new interactions which lead to violations of the universality of free fall (UFF). We discuss progress towards a proposed dual matter-wave interferometer which will measure the differential acceleration of 6Li and 7Li atoms. The difference in the baryon-to-lepton number ratio and nuclear binding energy for these two species gives higher sensitivity than many other proposed tests of UFF. However, the high thermal velocity of lithium, due to its light mass, leads to large atom loss in a traditional interferometer. To overcome this, an optical lattice will confine the lithium atoms during the interferometry sequence. Manipulations of the optical lattice will split the matter waves and hold the arms of the interferometer apart for many seconds in a compact apparatus. This large separation time leads to an anticipated accuracy of 10-14 g in the differential acceleration. We discuss possible systematic effects and show that many will be common mode to the two species. Finally we will review technical progress on the experiment and recent investigations into novel cooling techniques for lithium.

  13. The ^12C(^7Li,^6Li)^13C Transfer Reaction

    NASA Astrophysics Data System (ADS)

    Bartosz, E. E.; Keeley, N.; Kemper, K. W.

    2001-04-01

    We present the first complete set of analysing powers, including all third rank ones, for a ^7Li induced transfer reaction. Data were obtained for transfers to the 1/2^-, 1/2^+ and 5/2^+ states of ^13C at 0.0, 3.09 and 3.85 MeV excitation energies respectively, induced by a 34 MeV polarised ^7Li beam. This experiment was motivated by the complete failure of previous DWBA and CCBA calculations to describe transfers to the 1/2^+ state (K.W. Kemper, et al./, Phys. Rev. C 38, 2664 (1988).). Extensive coupled-discretised-continuum-channels (CDCC) calculations using cluster-folding (CF) model form-factors have been carried out and show that the failure to describe the 1/2^+ data is not a result of a dynamical effect.

  14. Prediction of {sup 2}D Rydberg energy levels of {sup 6}Li and {sup 7}Li based on very accurate quantum mechanical calculations performed with explicitly correlated Gaussian functions

    SciTech Connect

    Bubin, Sergiy; Sharkey, Keeper L.; Adamowicz, Ludwik

    2013-04-28

    Very accurate variational nonrelativistic finite-nuclear-mass calculations employing all-electron explicitly correlated Gaussian basis functions are carried out for six Rydberg {sup 2}D states (1s{sup 2}nd, n= 6, Horizontal-Ellipsis , 11) of the {sup 7}Li and {sup 6}Li isotopes. The exponential parameters of the Gaussian functions are optimized using the variational method with the aid of the analytical energy gradient determined with respect to these parameters. The experimental results for the lower states (n= 3, Horizontal-Ellipsis , 6) and the calculated results for the higher states (n= 7, Horizontal-Ellipsis , 11) fitted with quantum-defect-like formulas are used to predict the energies of {sup 2}D 1s{sup 2}nd states for {sup 7}Li and {sup 6}Li with n up to 30.

  15. Trojan horse particle invariance studied with the {sup 6}Li(d,{alpha}){sup 4}He and {sup 7}Li(p,{alpha}){sup 4}He reactions

    SciTech Connect

    Pizzone, R. G.; Spitaleri, C.; Lamia, L.; Cherubini, S.; La Cognata, M.; Puglia, S. M. R.; Rapisarda, G. G.; Romano, S.; Sergi, M. L.; Bertulani, C.; Mukhamedzhanov, A.; Blokhintsev, L.; Burjan, V.; Hons, Z.; Kroha, V.; Mrazek, J.; Piskor, S.; Kiss, G. G.; Li, C.; Tumino, A.

    2011-04-15

    The Trojan horse nucleus invariance for the binary reaction cross section extracted from the Trojan horse reaction was tested using the quasifree {sup 3}He({sup 6}Li,{alpha}{alpha})H and {sup 3}He({sup 7}Li,{alpha}{alpha}){sup 2}H reactions. The cross sections for the {sup 6}Li(d,{alpha}){sup 4}He and {sup 7}Li(p,{alpha}){sup 4}He binary processes were extracted in the framework of the plane wave approximation. They are compared with direct behaviors as well as with cross sections extracted from previous indirect investigations of the same binary reactions using deuteron as the Trojan horse nucleus instead of {sup 3}He. The very good agreement confirms the applicability of the plane wave approximation which suggests the independence of the binary indirect cross section on the chosen Trojan horse nucleus, at least for the investigated cases.

  16. HOTSPUR progress report: neutron source spectrum characterization, and /sup 6/Li(n,x. cap alpha. ) and /sup 7/Li(n,x. cap alpha. ) cross section determination

    SciTech Connect

    Goldberg, E.; Haight, R.

    1984-04-02

    As a prerequisite to high accuracy measurements involving the bulk configuration of /sup 6/LiD we must have a good grasp of the details of the RTNS-I neutron source energy spectrum. Experiments to this end involving neutron yield vs deuteron energy, ratios of foil activation of selected elements, and pulse height distributions of a Si surface barrier detector are described. With this knowledge, the /sup 4/He-production cross sections for /sup 6/Li and /sup 7/Li are found experimentally to be 0.512b and 0.336b, respectively, at anti E/sub N/ = 15.0 MeV in free-field geometry. 14 references.

  17. Coincident emission of neutrons and charged particles after π- absorption in 6Li, 7Li, 12C, 59Co and 197Au

    NASA Astrophysics Data System (ADS)

    Heusi, P.; Isaak, H. P.; Pruys, H. S.; Engfer, R.; Hermes, E. A.; Kozlowski, T.; Sennhauser, U.; Walter, H. K.

    1983-10-01

    Energy spectra d 3W/d E1 d E2 d cos ϑ of neutron-neutron and neutron-charged particle pairs (nn, np, nd, nt) emitted after the absorption of stopped negative pions in 6Li, 7Li, 12C, 59Co and 197Au have been measured for opening angles between 50° and 180°. Particle pairs emitted from light nuclei without energy loss due to final-state interactions were identified by the energy balance. Pion absorption on two nucleons (quasi-deuteron mechanism) was found to be the main process. The yields of nucleon pairs from quasi-free absorption on a quasi-deuteron are 0.52 ± 0.09 per π-stop, 0.57 ± 0.10 per π-stop and 0.19 ± 0.04 per π-stop for 6Li, 7Li and 12C, respectively. The ratio R of np to pp pairs that absorb the pion was determined for quasi-free absorption on p-shell nucleons of 12C: R(p-shell) = 6.3 ± 1.4. For pion absorption on s-shell nucleons of lithium lower limits R(s-shell) > 4.4 for 6Li and R(s-shell) > 7.8 for 7Li were determined. These values are larger than the statistical ratios Rstat = 2 N/( Z - 1) of np to pp pairs in the nucleus. Lower limits for the probability for pion absorption on heavier clusters ( 3He, α) are W(hc) > 0.16 per π-stop for 6Li, W(hc) > 0.11 per π-stop for 7Li and W( α) > 0.01 per π-stop for 12C. The shape of the energy spectra of pairs emitted directly after quasi-free absorption on 2 or 4 nucleons could be explained by a simple model for the momentum distribution of the absorbing nucleons. The results are in agreement with the parameters of the momentum distributions known from other reactions. Energy spectra and opening-angle distributions were compared with the intranuclear cascade calculations of Chiang, Hüfner and Hachenberg. For 59Co and 197Au the spectra are strongly influenced by the final-state interactions; lower limits of R > 1.8 for 59Co and R > 2.5 for 197Au were determined.

  18. All-optical production of dual Bose-Einstein condensates of paired fermions and bosons with 6Li and 7Li

    NASA Astrophysics Data System (ADS)

    Ikemachi, Takuya; Ito, Aki; Aratake, Yukihito; Chen, Yiping; Koashi, Masato; Kuwata-Gonokami, Makoto; Horikoshi, Munekazu

    2017-01-01

    We report the first all-optical production of dual Bose-Einstein condensates (BECs) of paired 6Li (fermion) and one spin state of 7Li (boson) at the magnetic field where the s-wave interactions between fermions are resonant. Fermions are cooled efficiently by evaporative cooling and they serve as coolant for bosons. As a result, the dual condensates can be achieved by using a simple experimental apparatus and procedures, as in the case of the all-optical production of a single BEC. We show that the all-optical method enables us to realize variety of ultracold Bose-Fermi mixtures.

  19. The use of 6Li{7Li}-REDOR NMR spectroscopy to compare the ionic conductivities of solid-state lithium ion electrolytes.

    PubMed

    Spencer, T L; Plagos, N W; Brouwer, D H; Goward, G R

    2014-02-14

    Garnet-like solid-state electrolyte materials for lithium ion batteries are promising replacements for the currently-used liquid electrolytes. This work compares the temperature dependent Li(+) ion hopping rate in Li6BaLa2M2O12 (M = Ta, Nb) using solid-state (6)Li{(7)Li}-REDOR NMR. The slope of the (6)Li{(7)Li}-REDOR curve is highly temperature dependent in these two phases, and a comparison of the changes of the REDOR slopes as a function of temperature has been used to evaluate the Li(+) ion dynamics. Our results indicate that the Nb phase has a higher overall ionic conductivity in the range of 247 K to 350 K, as well as a higher activation energy for lithium ion hopping than the Ta counterpart. For appropriate relative timescales of the dipolar couplings and ion transport processes, this is shown to be a facile method to compare ion dynamics among similar structures.

  20. Parsec-scale Variations in the 7Li i/6Li i Isotope Ratio Toward IC 348 and the Perseus OB 2 Association

    NASA Astrophysics Data System (ADS)

    Knauth, D. C.; Taylor, C. J.; Ritchey, A. M.; Federman, S. R.; Lambert, D. L.

    2017-01-01

    Measurements of the lithium isotopic ratio in the diffuse interstellar medium from high-resolution spectra of the Li i λ6708 resonance doublet have now been reported for a number of lines of sight. The majority of the results for the 7Li/6Li ratio are similar to the solar system ratio of 12.2, but the line of sight toward o Per, a star near the star-forming region IC 348, gave a ratio of about two, the expected value for gas exposed to spallation and fusion reactions driven by cosmic rays. To examine the association of IC 348 with cosmic rays more closely, we measured the lithium isotopic ratio for lines of sight to three stars within a few parsecs of o Per. One star, HD 281159, has 7Li/6Li ≃ 2 confirming production by cosmic rays. The lithium isotopic ratio toward o Per and HD 281159 together with published analyses of the chemistry of interstellar diatomic molecules suggest that the superbubble surrounding IC 348 is the source of the cosmic rays. Based on observations obtained with the Hobby-Eberly Telescope, which is a joint project of the University of Texas at Austin, the Pennsylvania State University, Ludwig-Maximilians-Universität München, and Georg-August-Universität Göttingen.

  1. New results on P -odd asymmetry of γ -quanta emission in 10B(n, α)7Li* rightarrow γ + 7Li(g.s.) nuclear reaction

    NASA Astrophysics Data System (ADS)

    Vesna, V. A.; Gledenov, Yu. M.; Nesvizhevsky, V. V.; Sedyshev, P. V.; Shulgina, E. V.

    2011-03-01

    A series of ultra-sensitive experiments has been carried out in 2001-2009 at the ILL measuring P -odd asymmetry in γ -quanta emission in the nuclear reaction 10B ( n, α) 7Li* rightarrow γ + 7Li(g.s.) with polarized cold neutrons. The resulting value of the asymmetry coefficient is ensuremath α_{P-odd}= +(0.0 ± 2.6_{stat} ± 1.1_{syst}) × 10^{-8} . These experiments profited from high-intensity PF1B neutron facility and a new version of the integral measuring method: for decreasing experimental uncertainties, the frequency of neutron spin-flip was higher than a typical reactor power noise frequency. Using the new value, we constrain the weak neutral current constant in the cluster model framework to ensuremath f_{π}^{^{10}B} ≤ 0.6 × 10^{-7} (at 90% c.l.). This constraint agrees with that following from the nuclear reaction 6Li ( n, α) 3H : ensuremath f_{π}^{6Li} ≤ 1.1 × 10^{-7} (at 90% c.l.). However, they both contradict the "best" value in the quark model by Desplanques, Donoughe, and Holstein ensuremath f_{π}^{DDH}=4.6\\cdot 10^{-7} . We invite experts in the field to contribute to the theoretical analysis of the problem.

  2. Metals, a Plasma of the Poor Man: Electron Screening in 7Li(p,{alpha}){alpha} and 6Li(p,{alpha})3He for Different Environments

    SciTech Connect

    Rolfs, C.

    2006-05-24

    The electron screening in the 7Li(p,{alpha}){alpha} reaction has been studied at Ep = 30 to 100 keV for different environments: Li2WO4 insulator, Li metal, and PdLi alloys. For the insulator a screening potential energy of Ue = 185{+-}150 eV was observed, consistent with previous work and the atomic adiabatic limit. However, for the Li metal and the PdLi alloys we find large values of Ue = 1280{+-}60 and 3790{+-}330 eV, respectively: the values can be explained by the plasma model of Debye applied to the quasi-free metallic electrons in these samples. Similar results have been found for the 6Li(p,{alpha})3He reaction supporting the hypothesis of the isotopic independence of the electron screening effect. The data together with previous studies of d(d,p)t and 9Be(p,{alpha})6Li in metals verify the Debye model scaling Ue {proportional_to} Zt (charge number of target)

  3. THE RADIATIVE NEUTRON CAPTURE ON 2H, 6Li, 7Li, 12C AND 13C AT ASTROPHYSICAL ENERGIES

    NASA Astrophysics Data System (ADS)

    Dubovichenko, Sergey; Dzhazairov-Kakhramanov, Albert; Burkova, Natalia

    2013-05-01

    The continued interest in the study of radiative neutron capture on atomic nuclei is due, on the one hand, to the important role played by this process in the analysis of many fundamental properties of nuclei and nuclear reactions, and, on the other hand, to the wide use of the capture cross-section data in the various applications of nuclear physics and nuclear astrophysics, and, also, to the importance of the analysis of primordial nucleosynthesis in the Universe. This paper is devoted to the description of results for the processes of the radiative neutron capture on certain light atomic nuclei at thermal and astrophysical energies. The consideration of these processes is done within the framework of the potential cluster model (PCM), general description of which was given earlier. The methods of usage of the results obtained, based on the phase shift analysis intercluster potentials, are demonstrated in calculations of the radiative capture characteristics. The considered capture reactions are not part of stellar thermonuclear cycles, but involve in the basic reaction chain of primordial nucleosynthesis in the course of the Universe formation.

  4. Effect of the nuclear medium on α -cluster excitation in 6Li

    NASA Astrophysics Data System (ADS)

    Yamagata, Tamio; Nakayama, Shintaro; Akimune, Hidetoshi; Miyamoto, Syuji

    2017-04-01

    The giant dipole resonance (GDR) in 6Li was investigated via the 6Li(γ ,x n ) reactions by using quasi-mono-energy γ rays in an energy range from 4.9 to 53.6 MeV. The γ rays were generated via Compton backscattering of Nd laser photons with relativistic energy electrons in an electron storage ring, NewSUBARU. The energy resolution in a full width at half maximum of γ ray was simulated to be 5 % at 50 MeV. Photoneutrons were detected with a 4 π -type neutron detector consisting of 41 3He-gas proportional counters. The (γ ,n ) cross sections were dominant, while the (γ ,2 n ) and (γ ,3 n ) cross sections were negligibly small. The energy integral of photoneutron cross sections up to 53.6 MeV was 59 MeV mb , which exhausted 65 % of the Thomas-Reiche-Kuhn sum rule. The GDR in 6Li was found to consist of mainly two components. The peak energy and the width for the low-energy component were Er=12 ±1 MeV and Γ =21 ±2 MeV . Those for the high-energy component were Er=33 ±2 MeV and Γ =30 ±2 MeV. The low-energy component corresponded to the GDR in 6Li. The high-energy component was inferred to be the GDR owing to an α -cluster excitation in 6Li. The existence of this component was recently proposed and was suggested by the experimental studies of the (p ,p') , (3He,t ) , and (7Li,7Be) reactions. The observed resonance shape of the high-energy component was well reproduced by modifying the GDR shape of a theoretical prediction for 4He at Er=26 MeV with Γ =20 MeV ; with increasing the excitation energy by 7 MeV (Q value was more negative), widening the width by 1.5 ±0.1 times, and decreasing a peak height by 0.29 ±0.02 times. As a result, the magnitude of the energy integral of the cross sections for the high-energy component observed in the present work was 0.86 ±0.06 times that in the theoretical prediction of the 4He(γ ,n ) reaction. It is a well-known fact that a frequency of a vibrating system is inversely proportional to the size of the system. We

  5. Lithium abundance and 6Li/7Li ratio in the active giant HD 123351. I. A comparative analysis of 3D and 1D NLTE line-profile fits

    NASA Astrophysics Data System (ADS)

    Mott, A.; Steffen, M.; Caffau, E.; Spada, F.; Strassmeier, K. G.

    2017-08-01

    Context. Current three-dimensional (3D) hydrodynamical model atmospheres together with detailed spectrum synthesis, accounting for departures from local thermodynamic equilibrium (LTE), permit to derive reliable atomic and isotopic chemical abundances from high-resolution stellar spectra. Not much is known about the presence of the fragile 6Li isotope in evolved solar-metallicity red giant branch (RGB) stars, not to mention its production in magnetically active targets like HD 123351. Aims: A detailed spectroscopic investigation of the lithium resonance doublet in HD 123351 in terms of both abundance and isotopic ratio is presented. From fits of the observed spectrum, taken at the Canada-France-Hawaii telescope, with synthetic line profiles based on 1D and 3D model atmospheres, we seek to estimate the abundance of the 6Li isotope and to place constraints on its origin. Methods: We derive the lithium abundance A(Li) and the 6Li/7Li isotopic ratio by fitting different synthetic spectra to the Li-line region of a high-resolution CFHT spectrum (R = 120 000, S/N = 400). The synthetic spectra are computed with four different line lists, using in parallel 3D hydrodynamical CO5BOLD and 1D LHD model atmospheres and treating the line formation of the lithium components in non-LTE (NLTE). The fitting procedure is repeated with different assumptions and wavelength ranges to obtain a reasonable estimate of the involved uncertainties. Results: We find A(Li) = 1.69 ± 0.11 dex and 6Li/7Li = 8.0 ± 4.4% in 3D-NLTE, using the line list of Meléndez et al. (2012, A&A, 543, A29), updated with new atomic data for V i, which results in the best fit of the lithium line profile of HD 123351. Two other line lists lead to similar results but with inferior fit qualities. Conclusions: Our 2σ detection of the 6Li isotope is the result of a careful statistical analysis and the visual inspection of each achieved fit. Since the presence of a significant amount of 6Li in the atmosphere of a cool

  6. New observations and mass-reduced analyses of the laser-excited fluorescence of the B1Π u- X1Σ g+ bands of the 6Li 7Li molecule

    NASA Astrophysics Data System (ADS)

    Verma, K. K.; Koch, M. E.; Stwalley, W. C.

    1981-06-01

    An Ar + laser at 4579 Å is used to excite the B1Π u- X1Σ g+ fluorescence of the 6Li 7Li molecule in a crossed heat pipe oven. The spectrum in the region 4400-6300 Å is recorded photoelectrically with an emphasis on the observation of higher vibrational levels in the ground state close to the dissociation limit. P and R doublets corresponding to v″ ≤ 26 originating from the ( v' = 13, J' = 19) level are observed and identified using mass-reduced quantum numbers. Two additional 6Li 7Li series, known from earlier work of Velasco, Ottinger, and Zare, are also analyzed. These data are used to construct effective Rydberg-Klein-Rees (RKR) potentials for specific J″ (=9, 19) quantum numbers of the ground state and from them the true (rotationless) potential energy curve (for X1Σ g+) is derived. This extends the previously known curve of Li 2 from 4.28 to 5.18 Å (outer turning point); this turning point corresponds to an energy which is approximately 88% of the dissociation energy, which is estimated here to be 8516 ± 18 cm -1.

  7. The use of enriched 6Li and 7Li Lif:Mg,Cu,P glass-rod thermoluminescent dosemeters for linear accelerator out-of-field radiation dose measurements.

    PubMed

    Takam, R; Bezak, E; Liu, G; Marcu, L

    2012-06-01

    (6)LiF:Mg,Cu,P and (7)LiF:Mg,Cu,P glass-rod thermoluminescent dosemeters (TLDs) were used for measurements of out-of-field photon and neutron doses produced by Varian iX linear accelerator. Both TLDs were calibrated using 18-MV X-ray beam to investigate their dose-response sensitivity and linearity. CR-39 etch-track detectors (Luxel+, Landauer) were employed to provide neutron dose data to calibrate (6)LiF:Mg,Cu,P TLDs at various distances from the isocentre. With cadmium filters employed, slow neutrons (<0.5 eV) were distinguished from fast neutrons. The average in-air photon dose equivalents per monitor unit (MU) ranged from 1.5±0.4 to 215.5±94.6 μSv at 100 and 15 cm from the isocentre, respectively. Based on the cross-calibration factors obtained with CR-39 etch-track detectors, the average in-air fast neutron dose equivalents per MU range from 10.6±3.8 to 59.1±49.9 μSv at 100 and 15 cm from the isocentre, respectively. Contribution of thermal neutrons to total neutron dose equivalent was small: 3.1±7.2 μSv per MU at 15 cm from the isocentre.

  8. TU-F-BRE-07: In Vivo Neutron Detection in Patients Undergoing Stereotactic Ablative Radiotherapy (SABR) for Primary Kidney Cancer Using 6Li and 7Li Enriched TLD Pairs

    SciTech Connect

    Lonski, P; Kron, T; Franich, R; Keehan, S; Siva, S; Taylor, M

    2014-06-15

    Purpose: Stereotactic ablative radiotherapy (SABR) for primary kidney cancer often involves the use of high-energy photons combined with a large number of monitor units. While important for risk assessment, the additional neutron dose to untargeted healthy tissue is not accounted for in treatment planning. This work aims to detect out-of-field neutrons in vivo for patients undergoing SABR with high-energy (>10 MV) photons and provides preliminary estimates of neutron effective dose. Methods: 3 variations of high-sensitivity LiF:Mg,Cu,P thermoluminescent dosimeter (TLD) material, each with varying {sup 6}Li / {sup 7}Li concentrations, were used in custom-made Perspex holders for in vivo measurements. The variation in cross section for thermal neutrons between Li isotopes was exploited to distinguish neutron from photon signal. Measurements were made out-of-field for 7 patients, each undergoing 3D-conformal SABR treatment for primary kidney cancer on a Varian 21iX linear accelerator. Results: In vivo measurements show increased signal for the {sup 6}Li enriched material for patients treated with 18 MV photons. Measurements on one SABR patient treated using only 6 MV showed no difference between the 3 TLD materials. The out-of-field photon signal decreased exponentially with distance from the treatment field. The neutron signal, taken as the difference between {sup 6}Li enriched and {sup 7}Li enriched TLD response, remains almost constant up to 50 cm from the beam central axis. Estimates of neutron effective dose from preliminary TLD calibration suggest between 10 and 30 mSv per 1000 MU delivered at 18 MV for the 7 patients. Conclusion: TLD was proven to be a useful tool for the purpose of in vivo neutron detection at out-of-field locations. Further work is required to understand the relationship between TL signal and neutron dose. Dose estimates based on preliminary TLD calibration in a neutron beam suggest the additional neutron dose was <30 mSv per 1000 MU at 18 MV.

  9. {sup 7}Li(p,n) NUCLEAR DATA LIBRARY FOR INCIDENT PROTON ENERGIES TO 150 MEV

    SciTech Connect

    S. MASHNIK; ET AL

    2000-11-01

    Researchers at Los Alamos National Laboratory are considering the possibility of using the Low Energy Demonstration Accelerator (LEDA), constructed at LANSCE for the Accelerator Production of Tritium program (APT), as a neutron source. Evaluated nuclear data are needed for the p+{sup 7}Li reaction, to predict neutron production from thin and thick lithium targets. In this report we describe evaluation methods that make use of experimental data, and nuclear model calculations, to develop an ENDF-formatted data library for incident protons with energies up to 150 MeV. The important {sup 7}Li(p,n{sub 0}) and {sup 7}Li(p,n{sub 1}) reactions are evaluated from the experimental data, with their angular distributions represented using Lengendre polynomial expansions. The decay of the remaining reaction flux is estimated from GNASH nuclear model calculations. This leads to the emission of lower-energy neutrons and other charged particles and gamma-rays from preequilibrium and compound nucleus decay processes. The evaluated ENDF-data are described in detail, and illustrated in numerous figures. We also illustrate the use of these data in a representative application by a radiation transport simulation with the code MCNPX.

  10. The cosmological {sup 7}Li problem from a nuclear physics perspective

    SciTech Connect

    Broggini, C.; Canton, L.; Fiorentini, G.; Villante, F.L. E-mail: luciano.canton@pd.infn.it E-mail: francesco.villante@lngs.infn.it

    2012-06-01

    The primordial abundance of {sup 7}Li as predicted by Big Bang Nucleosynthesis (BBN) is more than a factor 2 larger than what has been observed in metal-poor halo stars. Herein, we analyze the possibility that this discrepancy originates from incorrect assumptions about the nuclear reaction cross sections relevant for BBN. To do this, we introduce an efficient method to calculate the changes in the {sup 7}Li abundance produced by arbitrary (temperature dependent) modifications of the nuclear reaction rates. Then, considering that {sup 7}Li is mainly produced from {sup 7}Be via the electron capture process {sup 7}Be+e{sup −} → {sup 7}Li+ν{sub e}, we assess the impact of the various channels of {sup 7}Be destruction. Differently from previous analysis, we consider the role of unknown resonances by using a complete formalism which takes into account the effect of Coulomb and centrifugal barrier penetration and that does not rely on the use of the narrow-resonance approximation. As a result of this, the possibility of a nuclear physics solution to the {sup 7}Li problem is significantly suppressed. Given the present experimental and theoretical constraints, it is unlikely that the {sup 7}Be+n destruction rate is underestimated by the 2.5 factor required to solve the problem. We exclude, moreover, that resonant destruction in the channels {sup 7}Be+t and {sup 7}Be+{sup 3}He can explain the {sup 7}Li puzzle. New unknown resonances in {sup 7}Be+d and {sup 7}Be+α could potentially produce significant effects. Recent experimental results have ruled out such a possibility for {sup 7}Be+d. On the other hand, for the {sup 7}Be+α channel very favorable conditions are required. The possible existence of a partially suitable resonant level in {sup 11}C is studied in the framework of a coupled-channel model and the possibility of a direct measurement is considered.

  11. Error-systematics of determining simultaneously the (6 )Li /(7)Li and the (10)B/(11)B abundance ratios as Li(2)BO(2)(+): considerations for analyte elements of varying isotopic abundance patterns.

    PubMed

    Datta

    2000-09-15

    In the Li(2)BO(2)(+) ion beam method of isotopic analysis of elements, the (two) analyte isotopic abundance ratios (E( i)'s) are determined by solving a set of (two) simultaneous equations: f( i)(E( i)'s) = R( i) +/- delta( i), (i = 1, 2) where the R( i)'s are the measured isotopic molecular abundance ratios. We have shown recently that, in the process of solution of these equations, the experimental errors (delta( i)'s) are transformed into the actual errors of analysis, delta(E)'s, through some multiplication factors (MFs). For a given isotopic abundance distribution (IAD) of the Li(2)BO(2)(+) ions, the MFs are shown to depend on the combination of two molecular pairs (CTMPS) used as the monitor pairs for measurements, thereby indicating the requirement of careful selection of monitor pairs for avoiding large (propagated) errors in analysis. In this work, we study how the requirements for a correct analysis vary with the IADs of the elements to be analyzed. The results not only lay great emphasis on the need for proper selection, but also show that no CTMPS can be identified as the universal monitor pairs irrespective of molecular IAD. These observations are, moreover, independent of the actual isotopic abundances of the monitor ions and/or the achievable measurement accuracy (delta( i)). It is noted further that, depending on the IADs of the analyte elements and hence the specific IAD of the Li(2)BO(2)(+) ions, it may also happen that none of the different possible CTMPS really fits the criteria as the recommended monitor pairs, and then one has to ensure that the measurements are not only accurate but as perfect as possible (delta( i)'s --> 0) so as to achieve a reasonable accuracy in analysis. These findings are explained in terms of variations of MFs as a function of molecular IAD, and elaborated using experimental data. A comparative discussion on the determination of both (6)Li/(7)Li and (10)B/(11)B abundance ratios together, and that of either of them, as

  12. Depth profiling Li in electrode materials of lithium ion battery by 7Li(p,γ)8Be and 7Li(p,α)4He nuclear reactions

    NASA Astrophysics Data System (ADS)

    Sunitha, Y.; Kumar, Sanjiv

    2017-06-01

    A proton induced γ-ray emission method based on 7Li(p,γ)8Be proton capture reaction and a nuclear reaction analysis method involving 7Li(p,α)4He reaction are described for depth profiling Li in the electrode materials, graphite and lithium cobalt oxide for example, of a Li-ion battery. Depth profiling by 7Li(p,γ)8Be reaction is accomplished by the resonance at 441 keV and involves the measurement of 14.6 and 17.6 MeV γ-rays, characteristic of the reaction, by a NaI(Tl) detector. The method has a detection sensitivity of ˜0.2 at% and enables profiling up to a depth ≥20 μm with a resolution of ≥150 nm. The profiling to a fairly large depth is facilitated by the absence of any other resonance up to 1800 keV proton energy. The reaction has substantial off-resonance cross-sections. A procedure is outlined for evaluating the off-resonance yields. Interferences from fluorine and aluminium are major limitation of this depth profiling methodology. The depth profile measurement by 7Li(p,α)4He reaction, on the other hand, utilises 2-3 MeV protons and entails the detection of α-particles at 90° or 150° angles. The reaction exhibits inverse kinematics at 150°. This method, too, suffers interference from fluorine due to the simultaneous occurrence of 19F(p,α)16O reaction. Kinematical considerations show that the interference is minimal at 90° and thus is the recommended angle of detection. The method is endowed with a detection sensitivity of ˜0.1 at%, a depth resolution of ˜100 nm and a probing depth of about 30 μm in the absence and 5-8 μm in the presence of fluorine in the material. Both methods yielded comparable depth profiles of Li in the cathode (lithium cobalt oxide) and the anode (graphite) of a Li-ion battery.

  13. 6Li from Solar Flares.

    PubMed

    Ramaty; Tatischeff; Thibaud; Kozlovsky; Mandzhavidze

    2000-05-10

    By introducing a hitherto ignored 6Li producing process, due to accelerated 3He reactions with 4He, we show that accelerated particle interactions in solar flares produce much more 6Li than 7Li. By normalizing our calculations to gamma-ray data, we demonstrate that the 6Li produced in solar flares, combined with photospheric 7Li, can account for the recently determined solar wind lithium isotopic ratio, obtained from measurements in lunar soil, provided that the bulk of the flare-produced lithium is evacuated by the solar wind. Further research in this area could provide unique information on a variety of problems, including solar atmospheric transport and mixing, solar convection and the lithium depletion issue, and solar wind and solar particle acceleration.

  14. Big Bang 6Li nucleosynthesis studied deep underground (LUNA collaboration)

    NASA Astrophysics Data System (ADS)

    Trezzi, D.; Anders, M.; Aliotta, M.; Bellini, A.; Bemmerer, D.; Boeltzig, A.; Broggini, C.; Bruno, C. G.; Caciolli, A.; Cavanna, F.; Corvisiero, P.; Costantini, H.; Davinson, T.; Depalo, R.; Elekes, Z.; Erhard, M.; Ferraro, F.; Formicola, A.; Fülop, Zs.; Gervino, G.; Guglielmetti, A.; Gustavino, C.; Gyürky, Gy.; Junker, M.; Lemut, A.; Marta, M.; Mazzocchi, C.; Menegazzo, R.; Mossa, V.; Pantaleo, F.; Prati, P.; Rossi Alvarez, C.; Scott, D. A.; Somorjai, E.; Straniero, O.; Szücs, T.; Takacs, M.

    2017-03-01

    The correct prediction of the abundances of the light nuclides produced during the epoch of Big Bang Nucleosynthesis (BBN) is one of the main topics of modern cosmology. For many of the nuclear reactions that are relevant for this epoch, direct experimental cross section data are available, ushering the so-called "age of precision". The present work addresses an exception to this current status: the 2H(α,γ)6Li reaction that controls 6Li production in the Big Bang. Recent controversial observations of 6Li in metal-poor stars have heightened the interest in understanding primordial 6Li production. If confirmed, these observations would lead to a second cosmological lithium problem, in addition to the well-known 7Li problem. In the present work, the direct experimental cross section data on 2H(α,γ)6Li in the BBN energy range are reported. The measurement has been performed deep underground at the LUNA (Laboratory for Underground Nuclear Astrophysics) 400 kV accelerator in the Laboratori Nazionali del Gran Sasso, Italy. The cross section has been directly measured at the energies of interest for Big Bang Nucleosynthesis for the first time, at Ecm = 80, 93, 120, and 133 keV. Based on the new data, the 2H(α,γ)6Li thermonuclear reaction rate has been derived. Our rate is even lower than previously reported, thus increasing the discrepancy between predicted Big Bang 6Li abundance and the amount of primordial 6Li inferred from observations.

  15. Neutron Energy Spectra and Yields from the 7Li(p,n) Reaction for Nuclear Astrophysics

    NASA Astrophysics Data System (ADS)

    Tessler, M.; Friedman, M.; Schmidt, S.; Shor, A.; Berkovits, D.; Cohen, D.; Feinberg, G.; Fiebiger, S.; Krása, A.; Paul, M.; Plag, R.; Plompen, A.; Reifarth, R.

    2016-01-01

    Neutrons produced by the 7Li(p, n)7Be reaction close to threshold are widely used to measure the cross section of s-process nucleosynthesis reactions. While experiments have been performed so far with Van de Graaff accelerators, the use of RF accelerators with higher intensities is planned to enable investigations on radioactive isotopes. In parallel, high-power Li targets for the production of high-intensity neutrons at stellar energies are developed at Goethe University (Frankfurt, Germany) and SARAF (Soreq NRC, Israel). However, such setups pose severe challenges for the measurement of the proton beam intensity or the neutron fluence. In order to develop appropriate methods, we studied in detail the neutron energy distribution and intensity produced by the thick-target 7Li(p,n)7Be reaction and compared them to state-of- the-art simulation codes. Measurements were performed with the bunched and chopped proton beam at the Van de Graaff facility of the Institute for Reference Materials and Measurements (IRMM) using the time-of-flight (TOF) technique with thin (1/8") and thick (1") detectors. The importance of detailed simulations of the detector structure and geometry for the conversion of TOF to a neutron energy is stressed. The measured neutron spectra are consistent with those previously reported and agree well with Monte Carlo simulations that include experimentally determined 7Li(p,n) cross sections, two-body kinematics and proton energy loss in the Li-target.

  16. Analysis of 6Li Scattering at 240 MeV Using Different Nuclear Potentials

    NASA Astrophysics Data System (ADS)

    Al-Ghamdi, A. H.; Ibraheem, Awad A.

    2016-06-01

    Angular distributions of the elastic and inelastic scattering cross sections of 6Li projectile on different heavy ion target nuclei including the 24Mg, 28Si, 48Ca, 58Ni, 90Zr, and 116Sn at energy of 240 MeV have been analyzed by using two different folded potentials based on the CDM3Y6 and São Paulo potentials for the real part of the optical potential, while the imaginary parts have a phenomenological Woods-Saxon shape. Coupled channel calculations for the low-lying 2+ state at 1.369, 1.779, 3.832, 1.454, 2.186, and 1.29 MeV for 24Mg, 28Si, 48Ca, 58Ni, 90Zr, and 116Sn, respectively, have been carried out, and the best fit values for B(EL) with the above models have been extracted by fitting the inelastic scattering cross section and compared with the values of previous works. The total reaction cross section and real and imaginary volume integrals have also been investigated.

  17. Effect of compound nuclear reaction mechanism in 12C(6Li,d) reaction at sub-Coulomb energy

    NASA Astrophysics Data System (ADS)

    Mondal, Ashok; Adhikari, S.; Basu, C.

    2017-09-01

    The angular distribution of the 12C(6Li,d) reaction populating the 6.92 and 7.12 MeV states of 16O at sub-Coulomb energy (Ecm=3 MeV) are analysed in the framework of the Distorted Wave Born Approximation (DWBA). Recent results on excitation function measurements and backward angle angular distributions derive ANC for both the states on the basis of an alpha transfer mechanism. In the present work, we show that considering both forward and backward angle data in the analysis, the 7.12 MeV state at sub-Coulomb energy is populated from Compound nuclear process rather than transfer process. The 6.92 MeV state is however produced from direct reaction mechanism.

  18. 7Li-nuclear magnetic resonance observations of lithium insertion into coke carbon modified with mesophase-pitch

    NASA Astrophysics Data System (ADS)

    Sato, Yuichi; Tanuma, Ken-ichi; Takayama, Toshio; Kobayakawa, Koichi; Kawai, Takanobu; Yokoyama, Akira

    Lithium intercalation into coke carbon modified with mesophase-pitch and heat-treated at 800, 1000, and 3000°C was observed using solid-state 7Li-nuclear magnetic resonance ( 7Li-NMR) spectroscopy. It was found that the fully lithiated state charged to 0 V in the modified coke heat-treated at 3000°C showed a peak at about 45 ppm; on the other hand, two peaks appeared at about 45 and 16-17 ppm in the modified coke heat-treated below 1000°C. The peak appearing at 45 ppm indicated that Li-GIC is present in the first stage, and the peak at about 16-17 ppm indicated that the lithium stored in the modified part has an ionic character greater than in the coke part and is not a lithium cluster. The lithiated states charged to 0.1 and 0.2 V and discharged to 0.1, 0.2 and 1.5 V from the charged state (0 V) are also described.

  19. Investigation of {sup 6}Li + {sup 13}C scattering and observation of a nuclear quasi-rainbow

    SciTech Connect

    Dem`yanova, A.S.; Ogloblin, A.A.; Osadchii, O.Ya.

    1994-11-01

    Differential cross sections for elastic scattering of {sup 6}Li ions by {sup 13}C at E{sub c.m.s.} = 26 MeV are measured in the range of c.m.s. angles 14 - 163{degrees} at the Kurchatov Institute cyclotron in both direct and inverse kinematics by the {Delta}E-E telescope technique. A broad maximum in the angular distribution that is exhausted completely by the far component is observed at approximately 100{degrees}. The maximum is a typical manifestation of the nuclear rainbow and can be explained by the interference of waves arriving from the two branches of the deflection function (DF). However, for the potential chosen in this study, the DF has a singularity, and nuclear-rainbow scattering cannot formally take place because there is no finite scattering angle. The observed effect, which is referred to as a quasi-rainbow, demonstrates that the principal peculiarities of elastic scattering are the same in the two energy regions that are considered in a direct semiclassical approximation as corresponding to two fundamentally different phenomena: orbiting and the rainbow. 11 refs., 4 figs., 1 tab.

  20. Investigation of the Interaction of η-Mesons with an 6Li Nucleus Using the Nuclear Cluster Model

    NASA Astrophysics Data System (ADS)

    Adamov, E. V.; Egorov, M. V.; Fix, A. I.

    2017-02-01

    The problem of the interaction in the η-6Li system is solved. To solve this problem, we used the cluster model in which the 6Li nucleus is described as a bound state of a deuteron and an α-particle. The cluster approach allows one to reduce the many-body problem to the interaction in a system of three particles: η- d-α. To solve the corresponding three-body equations, we used the separable representation of two-body driving potentials. Calculated values of the η6Li scattering length are presented.

  1. First observation of P-odd asymmetry of α-particle emission in the 10B (n , α)7Li nuclear reaction

    NASA Astrophysics Data System (ADS)

    Gledenov, Yu. M.; Nesvizhevsky, V. V.; Sedyshev, P. V.; Shul'gina, E. V.; Szalanski, P.; Vesna, V. A.

    2017-06-01

    We present measurements of P-odd asymmetry of emission of α-particles in the 10B (n , α)7Li nuclear reaction, which are carried out using beams of polarized cold neutrons at Petersburg Nuclear Physics Institute (PNPI, Gatchina, Russia) and Institut Max von Laue - Paul Langevin (ILL, Grenoble, France) nuclear reactors. The α-particle detector is an ionization chamber with insensitive gaseous layer.

  2. The Application of U-Np Fuel and {sup 6}Li Burnable Poison for Space Reactors

    SciTech Connect

    Nikitin, Konstantin L.; Saito, Masaki; Artisyuk, Vladimir V.

    2003-11-15

    The possible application of {sup 6}Li as a burnable poison and U-Np nitride as a fuel for space nuclear reactors has been studied. The analysis was performed for an infinite lattice with a leakage in the form of buckling and (U-Np)N fuel with 20% uranium enrichment. The combination of {sup 7}Li as a coolant and {sup 6}Li as a burnable poison results in a favorable criticality behavior during burnup. The parameters taken into consideration include the different fuel and coolant compositions, the form of absorber material, and the various absorber mass and concentrations. It was found that absorption properties of {sup 6}Li allow reaching the burnup value up to 67 GWd/tHM while reactivity swing is comparable with {beta}{sub eff}. The corresponding reactor lifetime is {approx}10 to 30 yr.

  3. 7Li relaxation time measurements at very low magnetic field by 1H dynamic nuclear polarization

    NASA Astrophysics Data System (ADS)

    Zeghib, Nadir; Grucker, Daniel

    2001-09-01

    Dynamic nuclear polarization (DNP) of water protons was used to measure the relaxation time of lithium at very low magnetic field as a demonstration of the use of DNP for nuclei less abundant than water protons. Lithium (Li+) was chosen because it is an efficient treatment for manic-depressive illness, with an unknown action mechanism. After having recalled the theoretical basis of a three-spin system comprising two nuclei - the water proton of the solvent, the dissolved Li+ ion and the free electron of a free radical - we have developed a transient solution in order to optimize potential biological applications of Li DNP. The three-spin model has allowed computation of all the parameters of the system - the longitudinal relaxation rate per unit of free radical concentration, the dipolar and scalar part of the coupling between the nuclei and the electron, and the maximum signal enhancement achievable for both proton and lithium spins. All these measurements have been obtained solely through the detection of the proton resonance.

  4. Measurement of Nuclear Reaction Q-values with High Accuracy: 7Li(p, n)7Be

    NASA Astrophysics Data System (ADS)

    White, R. E.; Barker, P. H.; Lovelock, D. M. J.

    1985-01-01

    A technique is described for the measurement of nuclear reaction Q-values with an accuracy of a few parts in 105, in which the ultimate reference is a one-volt standard. As a test of the technique the accurately known threshold energy of the 7Li(p, n)7Be reaction, 1880.51 +/- 0.08 keV, has been remeasured. The value found using the present technique is 1880.443 +/- 0.020 keV, in good agreement with previous values. An attempt to see evidence for atomic excitation effects in the 27A1(p,n)27Si reaction is also discussed. This yielded a new value of 5803.73 +/- 0.12 keV for the threshold of this reaction, again in a good agreement with, but more accurate than, previous values. Further test measurements are summarized. The main application of the technique, in measurements related to the theory of weak interactions, is discussed briefly and the results obtained to date are presented.

  5. EFFECTS OF NUCLEAR INDUCED BREAKUP ON THE FUSION OF 6Li+12C AND 6He+12C SYSTEMS AROUND BARRIER ENERGIES

    NASA Astrophysics Data System (ADS)

    Duhan, Sukhvinder S.; Singh, Manjeet; Kharab, Rajesh

    2012-06-01

    We have studied the effects of nuclear induced breakup channel coupling on the fusion cross-section for 6Li+12C and 6He+12C systems in the near barrier energy regime using the dynamic polarization potential (DPP) approach. It has been found that there is enhancement in the fusion cross-section with respect to standard one-dimensional barrier penetration model in the below barrier energy regime while at energies above the barrier there is suppression of fusion cross-section with respect to simple barrier penetration model is observed. The agreement between data and predictions for 6Li+12C system improves significantly as a result of the inclusion of nuclear induced DPP.

  6. First direct measurement of the 2H(α,γ)6Li cross section at big bang energies and the primordial lithium problem.

    PubMed

    Anders, M; Trezzi, D; Menegazzo, R; Aliotta, M; Bellini, A; Bemmerer, D; Broggini, C; Caciolli, A; Corvisiero, P; Costantini, H; Davinson, T; Elekes, Z; Erhard, M; Formicola, A; Fülöp, Zs; Gervino, G; Guglielmetti, A; Gustavino, C; Gyürky, Gy; Junker, M; Lemut, A; Marta, M; Mazzocchi, C; Prati, P; Rossi Alvarez, C; Scott, D A; Somorjai, E; Straniero, O; Szücs, T

    2014-07-25

    Recent observations of (6)Li in metal poor stars suggest a large production of this isotope during big bang nucleosynthesis (BBN). In standard BBN calculations, the (2)H(α,γ)(6)Li reaction dominates (6)Li production. This reaction has never been measured inside the BBN energy region because its cross section drops exponentially at low energy and because the electric dipole transition is strongly suppressed for the isoscalar particles (2)H and α at energies below the Coulomb barrier. Indirect measurements using the Coulomb dissociation of (6)Li only give upper limits owing to the dominance of nuclear breakup processes. Here, we report on the results of the first measurement of the (2)H(α,γ)(6)Li cross section at big bang energies. The experiment was performed deep underground at the LUNA 400 kV accelerator in Gran Sasso, Italy. The primordial (6)Li/(7)Li isotopic abundance ratio has been determined to be (1.5 ± 0.3) × 10(-5), from our experimental data and standard BBN theory. The much higher (6)Li/(7)Li values reported for halo stars will likely require a nonstandard physics explanation, as discussed in the literature.

  7. Estimation of the nuclear distortion in the Coulomb breakup of 6Li into α + d in the field of 208Pb ion

    NASA Astrophysics Data System (ADS)

    Irgaziev, B. F.

    2014-04-01

    In this article the results of the evaluation of the contribution of nuclear disintegration, based on the basis of diffraction theory in the 208Pb(6Li, αd)208Pb Coulomb breakup at an energy of 156 MeV is presented. Comparison of the results of the calculation with the experimental data of Kiener et al. [Phys. Rev. C 44, 2195 (1991)] gives evidence for the dominance of the Coulomb dissociation mechanism and contribution of nuclear distortion, but essentially smaller than the value reported byHammache et al. [Phys. Rev. C 82, 065803 (2010)] and Sümmerer [Prog. Part. Nucl. Phys. 66, 298 (2011)].

  8. Nuclear structure with accurate chiral perturbation theory nucleon-nucleon potential: Application to 6Li and 10B

    SciTech Connect

    Navratil, P; Caurier, E

    2003-10-14

    The authors calculate properties of A = 6 system using the accurate charge-dependent nucleon-nucleon (NN) potential at fourth order of chiral perturbation theory. By application of the ab initio no-core shell model (NCSM) and a variational calculation in the harmonic oscillator basis with basis size up to 16 {h_bar}{Omega} they obtain the {sup 6}Li binding energy of 28.5(5) MeV and a converged excitation spectrum. Also, they calculate properties of {sup 10}B using the same NN potential in a basis space of up to 8 {h_bar}{Omega}. The results are consistent with results obtained by standard accurate NN potentials and demonstrate a deficiency of Hamiltonians consisting of only two-body terms. At this order of chiral perturbation theory three-body terms appear. It is expected that inclusion of such terms in the Hamiltonian will improve agreement with experiment.

  9. 6Li in metal-poor halo stars: real or spurious?

    NASA Astrophysics Data System (ADS)

    Steffen, M.; Cayrel, R.; Bonifacio, P.; Ludwig, H.-G.; Caffau, E.

    2010-03-01

    The presence of convective motions in the atmospheres of metal-poor halo stars leads to systematic asymmetries of the emergent spectral line profiles. Since such line asymmetries are very small, they can be safely ignored for standard spectroscopic abundance analysis. However, when it comes to the determination of the 6Li/7Li isotopic ratio, q(Li)=n(6Li)/n(7Li), the intrinsic asymmetry of the 7Li line must be taken into account, because its signature is essentially indistinguishable from the presence of a weak 6Li blend in the red wing of the 7Li line. In this contribution we quantity the error of the inferred 6Li/7Li isotopic ratio that arises if the convective line asymmetry is ignored in the fitting of the λ6707 Å lithium blend. Our conclusion is that 6Li/7Li ratios derived by Asplund et al. (2006), using symmetric line profiles, must be reduced by typically Δq(Li) ≈ 0.015. This diminishes the number of certain 6Li detections from 9 to 4 stars or less, casting some doubt on the existence of a 6Li plateau.

  10. Onset of nuclear structure effects in near-barrier elastic scattering of weakly bound nuclei: {sup 6}He and {sup 6}Li compared

    SciTech Connect

    Kucuk, Y.; Boztosun, I.; Keeley, N.

    2009-06-15

    The elastic scattering of the halo nucleus {sup 6}He from heavy targets at incident energies near the Coulomb barrier displays a marked deviation from the standard Fresnel-type diffraction behavior. This deviation is due to the strong Coulomb dipole breakup coupling produced by the Coulomb field of the heavy target, a specific feature of the nuclear structure of {sup 6}He. We have performed Continuum Discretized Coupled Channels calculations for the elastic scattering of {sup 6}He and {sup 6}Li from {sup 58}Ni, {sup 120}Sn, {sup 144}Sm, {sup 181}Ta and {sup 208}Pb targets in order to determine the range of Z{sub T} where this nuclear-structure specific coupling effect becomes manifest. We find that the strong Coulomb dipole breakup coupling effect is only clearly experimentally distinguishable for targets of Z{sub T}{approx_equal}80.

  11. Photodisintegration of 7Li with progeny nuclei in excited states

    NASA Astrophysics Data System (ADS)

    Wurtz, W. A.; Pywell, R. E.; Norum, B. E.; Kucuker, S.; Sawatzky, B. D.; Weller, H. R.; Stave, S.; Ahmed, M. W.

    2015-10-01

    We study the reaction channels 7Li+γ →n +6Li (2.19 ) , 7Li+γ →n +6Li(3.56 ) , and 7Li+γ →d +5He(1.27 )→n +d +4He by detecting neutrons produced by photodisintegration events. We find absolute cross sections and angular dependence for 7Li+γ →n +6Li(2.19 ) at photon energies 13 and 15 MeV and for 7Li+γ →n +67Li+γ →d +5He(1.27 )→n +d +4He we obtain an upper bound on its cross section at photon energies 12, 13, and 15 MeV.

  12. Coulomb-nuclear interference with {sup 6}Li: Isospin character of the 2{sub 1}{sup +} excitation in {sup 70,72,74}Ge

    SciTech Connect

    Barbosa, M.D.L.; Borello-Lewin, T.; Horodynski-Matsushigue, L.B.; Duarte, J.L.M.; Rodrigues, C.L.; Rodrigues, M.R.D.; Ukita, G.M.

    2005-02-01

    Ratios of B(E2) to B(IS2), that is, of the reduced quadrupole transition probabilities related, respectively, to charge and mass were extracted through Coulomb-nuclear interference (CNI) for the excitation of the 2{sub 1}{sup +} states in {sup 70,72,74}Ge, with a relative accuracy of less than 4%. For this purpose, the CNI angular distributions associated with the inelastic scattering of 28-MeV incident {sup 6}Li ions accelerated by the Sao Paulo Pelletron, and momentum analyzed by the Enge magnetic spectrograph were interpreted within the DWBA-DOMP approach (distorted wave approximation for the scattering process and deformed optical model for the structure representation) with global {sup 6}Li optical parameters. The present CNI results demonstrate an abrupt change in the B(E2)/B(IS2) ratio for {sup 74}Ge: although for {sup 70,72}Ge, values of the order of 1.0 or slightly higher were obtained, this ratio is 0.66 (7) for {sup 74}Ge. The heavier Ge isotope is thus one of the few nuclei that, so far, have been shown to present clear mixed symmetry components in their ground-state band.

  13. Search for solar axion emission from {sup 7}Li and D(p, γ){sup 3}He nuclear decays with the CAST γ-ray calorimeter

    SciTech Connect

    Andriamonje, S.; Aune, S.; Dafni, T.; Ferrer-Ribas, E.; Autiero, D.; Barth, K.; Davenport, M.; Lella, L. Di; Belov, A.; Beltrán, B.; Carmona, J.M.; Cebrián, S.; Bräuninger, H.; Englhauser, J.; Friedrich, P.; Collar, J.I.; Eleftheriadis, C.; Fanourakis, G.; Fischer, H.; Franz, J.; Collaboration: CAST collaboration; and others

    2010-03-01

    We present the results of a search for a high-energy axion emission signal from {sup 7}Li (0.478 MeV) and D(p, γ){sup 3}He (5.5 MeV) nuclear transitions using a low-background γ-ray calorimeter during Phase I of the CAST experiment. These so-called ''hadronic axions'' could provide a solution to the long-standing strong-CP problem and can be emitted from the solar core from nuclear M1 transitions. This is the first such search for high-energy pseudoscalar bosons with couplings to nucleons conducted using a helioscope approach. No excess signal above background was found.

  14. Excitation functions of {sup 6,7}Li+{sup 7}Li reactions at low energies

    SciTech Connect

    Prepolec, L.; Soic, N.; Blagus, S.; Miljanic, D.; Siketic, Z.; Skukan, N.; Uroic, M.; Milin, M.

    2009-08-26

    Differential cross sections of {sup 6,7}Li+{sup 7}Li nuclear reactions have been measured at forward angles (10 deg. and 20 deg.), using particle identification detector telescopes, over the energy range 2.75-10.00 MeV. Excitation functions have been obtained for low-lying residual-nucleus states. The well pronounced peak in the excitation function of {sup 7}Li({sup 7}Li,{sup 4}He){sup 10}Be(3.37 MeV,2{sup +}) at beam energy about 8 MeV, first observed by Wyborny and Carlson in 1971 at 0 deg., has been observed at 10 deg., but is less evident at 20 deg. The cross section obtained for the {sup 7}Li({sup 7}Li,{sup 4}He){sup 10}Be(g.s,0{sup +}) reaction is about ten times smaller. The well pronounced peak in the excitation function of {sup 7}Li({sup 7}Li,{sup 4}He){sup 10}Be(3.37 MeV,2{sup +}) reaction could correspond to excited states in {sup 14}C, at excitation energies around 30 MeV.

  15. Investigation of local symmetry in LiH3(SeO3)2 single crystals by 1H and 7Li nuclear magnetic resonance

    NASA Astrophysics Data System (ADS)

    Lim, Ae Ran

    2013-10-01

    The local environments of 1H and 7Li nuclei in LiH3(SeO3)2 crystals were investigated using FT NMR. The 7Li spectrum does changes from three resonance lines to one resonance line near Tm (=383 K). The variation in the splitting of the 7Li resonance lines with temperature indicates that the EFG at the Li sites produced by the (SeO3)2- groups varies with temperature. The changes in the temperature dependence of the intensity, line width, and spin-lattice relaxation time T1 near Tm for the 1H and 7Li nuclei coincide with the distortion of the structural framework surrounding each 1H and 7Li ion. Finally, the NMR results obtained here are compared to MH3(SeO3)2 (M = Na, K, and Cs) crystals previously reported.

  16. Investigation of Mechanical Activation on Li-N-H Systems Using 6Li Magic Angle Spinning Nuclear Magnetic Resonance at Ultra-High Field

    SciTech Connect

    Hu, Jian Zhi; Kwak, Ja Hun; Yang, Zhenguo; Osborn, William; Markmaitree, Tippawan; Shaw, Leonard D.

    2008-07-15

    Abstract The significantly enhanced spectral resolution in the 6Li MAS NMR spectra of Li-N-H systems at ultra-high field of 21.1 tesla is exploited, for the first time, to study the detailed electronic and chemical environmental changes associated with mechanical activation of Li-N-H system using high energy balling milling. Complementary to ultra-high field studies, the hydrogen discharge dynamics are investigated using variable temperature in situ 1H MAS NMR at 7.05 tesla field. The significantly enhanced spectral resolution using ultra-high filed of 21.1 tesla was demonstrated along with several major findings related to mechanical activation, including the upfield shift of the resonances in 6Li MAS spectra induced by ball milling, more efficient mechanical activation with ball milling at liquid nitrogen temperature than with ball milling at room temperature, and greatly enhanced hydrogen discharge exhibited by the liquid nitrogen ball milled samples.

  17. Effect of breakup coupling on fusion for 6,7Li+24Mg systems

    NASA Astrophysics Data System (ADS)

    Pradhan, M. K.; Mukherjee, A.; Dasmahapatra, B.

    2015-01-01

    To study the effect of breakup coupling on fusion we have derived fusion cross sections in the framework of continuum discretised coupled channels (CDCC) method using the coupled channels code FRESCO for the systems 6,7Li+24Mg. The CDCC predicted fusion cross sections for the 7Li+24Mg system agree well with the experimental fusion data whereas for the 6Li+24Mg system the agreement is reasonable at below barrier energies. However, within the limits of the present work no definite conclusion could be obtained from the quality of agreement at above barrier energies for the 6Li+24Mg system.

  18. Neutron-induced background by an α-beam incident on a deuterium gas target and its implications for the study of the 2H(α,γ)6Li reaction at LUNA

    NASA Astrophysics Data System (ADS)

    Anders, M.; Trezzi, D.; Bellini, A.; Aliotta, M.; Bemmerer, D.; Broggini, C.; Caciolli, A.; Costantini, H.; Corvisiero, P.; Davinson, T.; Elekes, Z.; Erhard, M.; Formicola, A.; Fülöp, Zs.; Gervino, G.; Guglielmetti, A.; Gustavino, C.; Gyürky, Gy.; Junker, M.; Lemut, A.; Marta, M.; Mazzocchi, C.; Menegazzo, R.; Prati, P.; Rossi Alvarez, C.; Scott, D.; Somorjai, E.; Straniero, O.; Szücs, T.

    2013-02-01

    The production of the stable isotope 6Li in standard Big Bang nucleosynthesis has recently attracted much interest. Recent observations in metal-poor stars suggest that a cosmological 6Li plateau may exist. If true, this plateau would come in addition to the well-known Spite plateau of 7Li abundances and would point to a predominantly primordial origin of 6Li , contrary to the results of standard Big Bang nucleosynthesis calculations. Therefore, the nuclear physics underlying Big Bang 6Li production must be revisited. The main production channel for 6Li in the Big Bang is the 2H(α,γ)6Li reaction. The present work reports on neutron-induced effects in a high-purity germanium detector that were encountered in a new study of this reaction. In the experiment, an α-beam from the underground accelerator LUNA in Gran Sasso, Italy, and a windowless deuterium gas target are used. A low neutron flux is induced by energetic deuterons from elastic scattering and, subsequently, the 2H(d,n)3He reaction. Due to the ultra-low laboratory neutron background at LUNA, the effect of this weak flux of 2-3MeV neutrons on well-shielded high-purity germanium detectors has been studied in detail. Data have been taken at 280 and 400keV α-beam energy and for comparison also using an americium-beryllium neutron source.

  19. The three-cluster structures in 7Li

    NASA Astrophysics Data System (ADS)

    Beck, R.; Krivec, R.; Mihailović, M. V.

    1981-06-01

    A cluster model for the description of light nuclei is investigated which includes the interplay of three-cluster structures with the two-cluster ones and allows molecule-like vibrations of clusters. It is applied to the nucleus 7Li in order to study the influence of the three-cluster structures of the type ( 4He- 2H-n) on the low-lying states previously described by two-cluster structures ( 4He- 3H) and ( 6Li-n). An effective central interaction is used in the calculation. The space of the wave functions is spanned by antisymmetrized products of two and three shell-model wave functions describing separated clusters. In the case of two-cluster configurations the separation s of the two shell-model potentials is used as the generator coordinate. In the case of three-cluster configurations with fragments A, B and C the separation s1 = sA - sB between the two shell-model potentials for fragments A and B is taken as one of the generator coordinates, the other one being the separation s 2 = s C - {(As A + Bs B) }/{(A + B)}. The cluster configurations are characterized also by the spins of fragments and their relative angular momenta ( L1 and L2). The rotational and the space inversion symmetry of the states is obtained by projecting the basic states onto the eigenspace of the operators J, M and the parity operator. An algebraic method based on an algorithm which expresses the rotation of the coordinates in terms of rotation of the generator coordinates is used. The structure of the nucleus 7Li is described by the two-cluster configuration ( 4He- 3H) and the three-cluster configurations ( 4He- 2H(I d)- n) , with Id = 0, 1, and the total spin I = {1}/{2}, {3}/{2}. In the wave function of three-cluster structure the pair of values L1 = 0, L2 = 1 only is included. The effective nuclear potential V2 of Volkov is used in the calculation. The energy of the ground state described by a single configuration of the two-cluster structure ( 4He- 3H) is lowered by 0.66 MeV when this

  20. Comprehensive analysis of large α yields observed in 6Li-induced reactions

    NASA Astrophysics Data System (ADS)

    Lei, Jin; Moro, Antonio M.

    2017-04-01

    Background: Large α yields have been reported over the years in reactions with 6Li and 7Li projectiles. Previous theoretical analyses have shown that the elastic breakup (EBU) mechanism (i.e., projectile breakup leaving the target in its ground state) is able to account only for a small fraction of the total α -inclusive breakup cross sections, pointing toward the dominance of nonelastic breakup (NEB) mechanisms. Purpose: We aim to provide a systematic study of the α -inclusive cross sections observed in nuclear reactions induced by 6Li projectiles. In addition to estimating the total α singles' cross sections, it is our goal to evaluate angular and energy distributions of these α particles and compare them with experimental data, when available. Method: We compute separately the EBU and NEB components of the inclusive breakup cross sections. For the former, we use the continuum-discretized coupled-channels (CDCC) method, which treats this mechanism to all orders. For the NEB part, we employ the model proposed by Ichimura et al. [Phys. Rev. C 32, 431 (1985)], 10.1103/PhysRevC.32.431, within the distorted-wave Born approximation (DWBA). Results: Overall, the sum of the computed EBU and NEB cross sections is found to reproduce very well the measured singles' cross sections. In all cases analyzed, we find that the inclusive breakup cross section is largely dominated by the NEB component. Conclusions: The presented method provides a global and systematic description of inclusive breakup reactions induced by 6Li projectiles. It provides also a natural explanation of the previously observed underestimation of the measured α yields by CDCC calculations. The method used here can be extended to other weakly bound projectiles, including halo nuclei.

  1. In situ 7Li and 133Cs nuclear magnetic resonance investigations on the role of Cs+ additive in lithium-metal deposition process

    SciTech Connect

    Hu, Jian Zhi; Zhao, Zhenchao; Hu, Mary Y.; Feng, Ju; Deng, Xuchu; Chen, Xilin; Xu, Wu; Liu, Jun; Zhang, Ji-Guang

    2016-02-01

    Application of Li metal electrode in rechargeable lithium battery is hindered by safety concerns due to dendritic growth on the electrode over several charge-discharge cycles. We have found previously that adding low concentration Cs+ in electrolytes can promote smooth deposition of lithium onto metal electrode during repeated charge-discharge cycling using idea Li|Cu battery without the using of a separator. In this work, quantitative in situ 7Li and 133Cs NMR investigations using real planar symmetric lithium battery cells with and without Cs+ additives were carried out. It is found that the deposited lithium atoms on electrodes are highly porous. Detailed analysis of the data were carried out by separating the 7Li signal from deposited lithium that was oriented parallel to the electrode surface with the signal from the Li-metal nanorodes oriented perpendicular or nearly perpendicular to the electrode surface. The results demonstrate that addition of Cs+ can significantly enhance both the formation of uniform Li nanorods, and the reversibility of electrode. In situ 133Cs NMR directly confirms that Cs+ migrates to the electrode to form a positively charged electrostatic shield during cycling process. Combining the quantitative analysis of the orientation dependent signals of deposited metal Li and previous ex-situ results, different Li deposition models are proposed. During cycling process, more “active” lithium participates in the Li transfer between the electrode and nanorods for the battery with Cs+, while for the battery without Cs+ more dead and thinker lithium rods are formed and Li transfer between dendrites from different electrodes dominates.

  2. REVISED BIG BANG NUCLEOSYNTHESIS WITH LONG-LIVED, NEGATIVELY CHARGED MASSIVE PARTICLES: UPDATED RECOMBINATION RATES, PRIMORDIAL {sup 9}Be NUCLEOSYNTHESIS, AND IMPACT OF NEW {sup 6}Li LIMITS

    SciTech Connect

    Kusakabe, Motohiko; Kim, K. S.; Cheoun, Myung-Ki; Kajino, Toshitaka; Kino, Yasushi; Mathews, Grant J. E-mail: kyungsik@kau.ac.kr E-mail: kajino@nao.ac.jp E-mail: gmathews@nd.edu

    2014-09-01

    We extensively reanalyze the effects of a long-lived, negatively charged massive particle, X {sup –}, on big bang nucleosynthesis (BBN). The BBN model with an X {sup –} particle was originally motivated by the discrepancy between the {sup 6,} {sup 7}Li abundances predicted in the standard BBN model and those inferred from observations of metal-poor stars. In this model, {sup 7}Be is destroyed via the recombination with an X {sup –} particle followed by radiative proton capture. We calculate precise rates for the radiative recombinations of {sup 7}Be, {sup 7}Li, {sup 9}Be, and {sup 4}He with X {sup –}. In nonresonant rates, we take into account respective partial waves of scattering states and respective bound states. The finite sizes of nuclear charge distributions cause deviations in wave functions from those of point-charge nuclei. For a heavy X {sup –} mass, m{sub X} ≳ 100 GeV, the d-wave → 2P transition is most important for {sup 7}Li and {sup 7,} {sup 9}Be, unlike recombination with electrons. Our new nonresonant rate of the {sup 7}Be recombination for m{sub X} = 1000 GeV is more than six times larger than the existing rate. Moreover, we suggest a new important reaction for {sup 9}Be production: the recombination of {sup 7}Li and X {sup –} followed by deuteron capture. We derive binding energies of X nuclei along with reaction rates and Q values. We then calculate BBN and find that the amount of {sup 7}Be destruction depends significantly on the charge distribution of {sup 7}Be. Finally, updated constraints on the initial abundance and the lifetime of the X {sup –} are derived in the context of revised upper limits to the primordial {sup 6}Li abundance. Parameter regions for the solution to the {sup 7}Li problem and the primordial {sup 9}Be abundances are revised.

  3. Revised Big Bang Nucleosynthesis with Long-lived, Negatively Charged Massive Particles: Updated Recombination Rates, Primordial 9Be Nucleosynthesis, and Impact of New 6Li Limits

    NASA Astrophysics Data System (ADS)

    Kusakabe, Motohiko; Kim, K. S.; Cheoun, Myung-Ki; Kajino, Toshitaka; Kino, Yasushi; Mathews, Grant. J.

    2014-09-01

    We extensively reanalyze the effects of a long-lived, negatively charged massive particle, X -, on big bang nucleosynthesis (BBN). The BBN model with an X - particle was originally motivated by the discrepancy between the 6, 7Li abundances predicted in the standard BBN model and those inferred from observations of metal-poor stars. In this model, 7Be is destroyed via the recombination with an X - particle followed by radiative proton capture. We calculate precise rates for the radiative recombinations of 7Be, 7Li, 9Be, and 4He with X -. In nonresonant rates, we take into account respective partial waves of scattering states and respective bound states. The finite sizes of nuclear charge distributions cause deviations in wave functions from those of point-charge nuclei. For a heavy X - mass, mX >~ 100 GeV, the d-wave → 2P transition is most important for 7Li and 7, 9Be, unlike recombination with electrons. Our new nonresonant rate of the 7Be recombination for mX = 1000 GeV is more than six times larger than the existing rate. Moreover, we suggest a new important reaction for 9Be production: the recombination of 7Li and X - followed by deuteron capture. We derive binding energies of X nuclei along with reaction rates and Q values. We then calculate BBN and find that the amount of 7Be destruction depends significantly on the charge distribution of 7Be. Finally, updated constraints on the initial abundance and the lifetime of the X - are derived in the context of revised upper limits to the primordial 6Li abundance. Parameter regions for the solution to the 7Li problem and the primordial 9Be abundances are revised.

  4. 6Li + ion implantation into polystyrene

    NASA Astrophysics Data System (ADS)

    Soares, M. R. F.; Alegaonkar, P.; Behar, M.; Fink, D.; Müller, M.

    2004-06-01

    100 keV 6Li + ions were implanted into polystyrene at fluences of 1 × 10 13 to 1 × 10 14 cm -2, and their depth distributions were determined by means of the neutron depth profiling technique. In no case the projectile ions are found to come to rest according to their predicted implantation profiles. Instead, they always undergo considerable migration. During the irradiation process this motion is influenced by the radiation damage, and during the subsequent annealing steps one deals with thermal diffusion. The implant redistribution is always found to be governed strongly by the self-created damage, insofar as both electronic and nuclear defects in the polymer act as trapping centers.

  5. Convection and 6Li in the atmospheres of metal-poor halo stars

    NASA Astrophysics Data System (ADS)

    Steffen, Matthias; Cayrel, R.; Bonifacio, P.; Ludwig, H.-G.; Caffau, E.

    2010-04-01

    Based on 3D hydrodynamical model atmospheres computed with the CO5BOLD code and 3D non-LTE (NLTE) line formation calculations, we study the effect of the convection-induced line asymmetry on the derived 6Li abundance for a range in effective temperature, gravity, and metallicity covering the stars of the Asplund et al. (2006) sample. When the asymmetry effect is taken into account for this sample of stars, the resulting 6Li/7Li ratios are reduced by about 1.5% on average with respect to the isotopic ratios determined by Asplund et al. (2006). This purely theoretical correction diminishes the number of significant 6Li detections from 9 to 4 (2σ criterion), or from 5 to 2 (3σ criterion). In view of this result the existence of a 6Li plateau appears questionable. A careful reanalysis of individual objects by fitting the observed lithium 6707 Å doublet both with 3D NLTE and 1D LTE synthetic line profiles confirms that the inferred 6Li abundance is systematically lower when using 3D NLTE instead of 1D LTE line fitting. Nevertheless, halo stars with unquestionable 6Li detection do exist even if analyzed in 3D-NLTE, the most prominent example being HD 84937.

  6. {sup 13}C, {sup 1}H, {sup 6}Li magic-angle spinning nuclear magnetic resonance, electron paramagnetic resonance, and Fourier transform infrared study of intercalation electrodes based in ultrasoft carbons obtained below 3100 K

    SciTech Connect

    Alcantara, R.; Madrigal, F.J.F.; Lavela, P.; Tirado, J.L.; Mateos, J.M.J.; Stoyanova, R.; Zhecheva, E.

    1999-01-01

    The past decade has seen an important development of materials for high-performance energy storage systems. Particularly, the field of electrode materials for advanced lithium batteries has attracted the interest of numerous researchers. Petroleum coke samples of different origins and heat treated at different temperatures below 3100 K have been studied by spectroscopic and electrochemical procedures. According to {sup 13}C and {sup 1}H magic-angle spinning (MAS) nuclear magnetic resonance (NMR), infrared (IR), and electron paramagnetic resonance (EPR) data, aromatic compounds and surface OH groups are present in green coke samples. The preparation of CMB (combustible) sample from 1673 K leads to a low-temperature graphitization process, as shown by the occurrence of multiphase products containing both turbostatic and graphitized solid. This process is accompanied by the loss of aromatic compounds and surface hydroxyls. The optimization of the lithium intercalation electrodes based in the green coke materials was carried out by thermal treatment at 1023 K under dynamic vacuum conditions. Such pretreatment of the electrode material leads to marked enhancement of reversible capacities without the higher temperatures usually required for other soft carbon materials. Finally, the results of {sup 6}Li MAS NMR and EPR have been correlated with the experimental determination of lithium diffusion coefficients and surface properties. On the basis of these results, spin resonance spectroscopies are found to be a powerful tool to discern between the different petroleum coke samples to select the active electrode material with best performance.

  7. New mass measurement of {sup 6}Li and ppb-level systematic studies of the Penning trap mass spectrometer TITAN

    SciTech Connect

    Brodeur, M.; Ettenauer, S.; Smith, M.; Dilling, J.; Brunner, T.; Champagne, C.; Lapierre, A.; Ringle, R.; Ryjkov, V. L.; Delheij, P.; Audi, G.; Lunney, D.

    2009-10-15

    The frequency ratio of {sup 6}Li to {sup 7}Li was measured using the TITAN Penning trap mass spectrometer. This measurement resolves a 16-ppb discrepancy between the {sup 6}Li mass of 6.015 122 795(16) u from the Atomic Mass Evaluation 2003 (AME03), which is based on a measurement by JILATRAP, and the more recent measurement of 6.015 122 890(40) u by SMILETRAP. Our measurement agrees with SMILETRAP and a more precise mass value for {sup 6}Li of 6.015 122 889(26) u is presented along with systematic evaluations of the measurement uncertainties. This result makes {sup 6}Li a solid anchor point for future mass measurements on highly charged ions with m/q{approx}6.

  8. Analogs of the giant dipole and spin-dipole resonances in {sup 4}He and in {alpha} clusters of {sup 6,7}Li studied by the {sup 4}He,{sup 6,7}Li({sup 7}Li,{sup 7}Be{gamma}) reactions

    SciTech Connect

    Nakayama, S.; Matsumoto, E.; Fushimi, K.; Hayami, R.; Kawasuso, H.; Yasuda, K.; Yamagata, T.; Akimune, H.; Ikemizu, H.; Asaji, S.; Ishida, T.; Kudoh, T.; Sagara, K.; Fujiwara, M.; Hashimoto, H.; Kawase, K.; Nakanishi, K.; Oota, T.; Yosoi, M.; Greenfield, M. B.

    2008-07-15

    We studied analogs of the giant dipole resonance (GDR) and spin-dipole resonance (SDR) in {sup 4}He and in the {alpha} clusters of {sup 6,7}Li via the ({sup 7}Li,{sup 7}Be{gamma}) reactions on {sup 4}He, {sup 6}Li, and {sup 7}Li at an incident energy of 455 MeV and at a scattering angle of 0 deg. by measuring spin-nonflip and spin-flip spectra. The reaction Q-values for the analogs of the GDR and SDR in the {alpha} clusters of {sup 6,7}Li were found to be more negative than those in {sup 4}He by 2.0{+-}0.5 MeV. The ratios of the cross section for the analog of the GDR to that for the analog of the SDR in {sup 4}He and in the {alpha} clusters of {sup 6}Li and {sup 7}Li were found to be the same within errors, 0.5{+-}0.1. The cross sections for the analogs of the GDR as well as those for the analogs of the SDR in the {alpha} clusters of {sup 6,7}Li were 0.6{approx}0.8 times smaller than those in {sup 4}He. These results suggest that excitations of {alpha} clusters embedded in nuclei are suppressed as compared with excitations of free {alpha} particles.

  9. Destructions of 7Be and 7Li in Big Bang nucleosynthesis through reactions with exotic long-lived sub-strongly interacting massive particles

    NASA Astrophysics Data System (ADS)

    Kusakabe, Motohiko; Kawasaki, Masahiro

    2012-11-01

    An observed plateau abundance of 7Li in metal-poor halo stars indicates its primordial origin. The 7Li abundances are about a factor of three smaller than that predicted in standard big bang nucleosynthesis (BBN) model. In addition, some of the stars possibly contain 6Li in abundances larger than standard BBN prediction. Particle models sometimes include heavy longlived colored particles which are confined in exotic strongly interacting massive particles (SIMPs). We have found reactions which destroy 7Be and 7Li during BBN in the scenario of BBN affected by a long-lived sub-strongly interactingmassive particle (sub-SIMP, X). The reactions are non radiative X captures of 7Be and 7Li which can operate if the X particle interacts with nuclei strongly enough to drive 7Be destruction but not strongly enough to form a bound state with 4He of relative angular momentum L = 1. The processes can be a cause of the 7Li problem. In this paper we suggest new possible reactions for 6Li production. Especially, a 6Li production through the deuteron capture of 4He bound to X can operate in the parameter region solving the 7Li problem.

  10. Destructions of {sup 7}Be and {sup 7}Li in Big Bang nucleosynthesis through reactions with exotic long-lived sub-strongly interacting massive particles

    SciTech Connect

    Kusakabe, Motohiko; Kawasaki, Masahiro

    2012-11-12

    An observed plateau abundance of {sup 7}Li in metal-poor halo stars indicates its primordial origin. The {sup 7}Li abundances are about a factor of three smaller than that predicted in standard big bang nucleosynthesis (BBN) model. In addition, some of the stars possibly contain {sup 6}Li in abundances larger than standard BBN prediction. Particle models sometimes include heavy longlived colored particles which are confined in exotic strongly interacting massive particles (SIMPs). We have found reactions which destroy {sup 7}Be and {sup 7}Li during BBN in the scenario of BBN affected by a long-lived sub-strongly interactingmassive particle (sub-SIMP, X). The reactions are non radiative X captures of {sup 7}Be and {sup 7}Li which can operate if the X particle interacts with nuclei strongly enough to drive {sup 7}Be destruction but not strongly enough to form a bound state with {sup 4}He of relative angular momentum L = 1. The processes can be a cause of the {sup 7}Li problem. In this paper we suggest new possible reactions for {sup 6}Li production. Especially, a {sup 6}Li production through the deuteron capture of {sup 4}He bound to X can operate in the parameter region solving the {sup 7}Li problem.

  11. 7Li NMR on Li intercalated carbon nanotubes

    NASA Astrophysics Data System (ADS)

    Schmid, M.; Goze-Bac, C.; Mehring, M.; Roth, S.

    2005-09-01

    Solid state 7Li Nuclear Magnetic Resonance (NMR) measurements were performed on lithium intercalated single wall carbon nanotubes (SWNT). The temperature dependence of the static spectra, as well as the spin-lattice relaxation behavior of the intercalated Li nuclei reveal two coexisting kinds of Li intercalation sites. Our results can be interpreted in terms of a staging phenomenon similar to graphite intercalation compounds (GIC).

  12. High-pressure superconducting phase diagram of 6Li: Isotope effects in dense lithium

    PubMed Central

    Schaeffer, Anne Marie; Temple, Scott R.; Bishop, Jasmine K.; Deemyad, Shanti

    2015-01-01

    We measured the superconducting transition temperature of 6Li between 16 and 26 GPa, and report the lightest system to exhibit superconductivity to date. The superconducting phase diagram of 6Li is compared with that of 7Li through simultaneous measurement in a diamond anvil cell (DAC). Below 21 GPa, Li exhibits a direct (the superconducting coefficient, α, Tc∝M−α, is positive), but unusually large isotope effect, whereas between 21 and 26 GPa, lithium shows an inverse superconducting isotope effect. The unusual dependence of the superconducting phase diagram of lithium on its atomic mass opens up the question of whether the lattice quantum dynamic effects dominate the low-temperature properties of dense lithium. PMID:25538300

  13. Analyzing Powers of (^6 Li,d) Reactions and the D State of ^6Li.

    NASA Astrophysics Data System (ADS)

    Veal, K. D.; Brune, C. R.; Geist, W. H.; Karwowski, H. J.; Ludwig, E. J.; Mendez, A. J.; Kozlowska, B.; Bartosz, E. E.; Cathers, P. D.; Drummer, T. L.; Kemper, K. W.; Eiró, A. M.; Santos, F. D.; Thompson, I. J.

    1997-10-01

    One way to quantify the D-state component of a light nucleus is in terms of η, the ratio of the D and S state asymptotic normalization constants. Calculations of tensor analyzing powers of transfer reactions induced by polarized ^6Li ions show considerable sensitivity to the magnitude and sign of η(^6Li). To this end, we have made measurements of the analyzing powers A_y, A_zz, and A_xz for the 0^+ gs and the lowest 2^+ state from (^6Li,d) reactions on ^58Ni and ^40Ca at E(^6Li) = 34 MeV. We have performed DWBA calculations that are in good agreement with the cross section and Ay data. Treating η(^6Li) as the only remaining adjustable fitting parameter, we have calculated a best fit value of η(^6Li) for each of the tensor analyzing power angular distributions. Preliminary estimates showing η(^6Li) to be smaller than previous determinations(D.R. Lehman, Colloque de Physique Suppl. n 22, 51), C6-47 (1990). will be presented.

  14. A direct measurement of the 6Li(n,t)4He cross section at sub-thermal neutron energy

    NASA Astrophysics Data System (ADS)

    Yue, A.; Dewey, M.; Gilliam, D.; Nico, J.; Greene, G.; Laptev, A.

    2014-09-01

    The thermal neutron capture cross section for the 6Li(n,t)4He reaction is an important neutron cross section standard. Yet few measurements of it have been performed and the ENDF/B-VII recommended value of (938 . 5 +/- 1 . 3) b is based heavily on measurements performed at higher energies. The first absolute, direct measurement of the 6Li(n,t)4He cross section at sub-thermal neutron energy has been performed at the NIST Center for Neutron Research. An alpha-gamma counter was used to measure the absolute neutron fluence of a monoenergetic neutron beam to sub-0.1% precision. The alpha-gamma counter used a thick, totally absorbing target of 10B-enriched boron carbide. The rate of absorbed neutrons was determined by counting the 478 keV 10B(n, γ)7Li gamma rays with calibrated high-purity germanium detectors. Simultaneously, the absolute rate of neutron-induced charged particles was measured for three thin 6Li targets of known density with a defined solid-angle counter. Using the known density of the 6Li targets and measurements of the rate of charged particles from the 6Li targets, the fluence of the neutron beam, and the energy of the neutron beam, we determine the 6Li(n,t)4He cross section at En = 3 . 3 meV to 0.3% uncertainty.

  15. Probing the fusion of 7Li with 64Ni at near-barrier energies

    NASA Astrophysics Data System (ADS)

    Shaikh, Md. Moin; Roy, Subinit; Rajbanshi, S.; Mukherjee, A.; Pradhan, M. K.; Basu, P.; Nanal, V.; Pal, S.; Shrivastava, A.; Saha, S.; Pillay, R. G.

    2016-04-01

    Background: The stable isotopes of Li, 6Li6 and 7Li, have two-body cluster structures of α +d and α +t with α -separation energies or breakup thresholds at 1.47 and 2.47 MeV, respectively. The weak binding of these projectiles introduces several new reaction channels not usually observed in the case of strongly bound projectiles. The impact of these breakup or breakup-like reaction channels on fusion, the dominant reaction process at near-barrier energies, with different target masses is of current interest. Purpose: Our purpose is to explore the fusion, at above and below the Coulmb barrier, of 7Li with 64Ni target in order to understand the effect of breakup or breakup-like processes with medium-mass target in comparison with 6Li, which has a lower breakup threshold. Measurement: The total fusion (TF) excitation of the weakly bound projectile 7Li with the medium-mass target 64Ni has been measured at the near-barrier energies (0.8 to 2 VB). The measurement was performed using the online characteristic γ -ray detection method. The complete fusion (CF) excitation function for the system was obtained using the x n -evaporation channels with the help of statistical model predictions. Results: At the above barrier energies CF cross sections exhibit an average suppression of about 6.5% compared to the one-dimensional barrier penetration model (1DBPM) predictions, while the model describes the measured TF cross section well. But below the barrier, both TF and CF show enhancements compared to 1DBPM predictions. Unlike 6Li, enhancement of CF for 7Li could not be explained by inelastic coupling alone. Conclusion: Whereas the σTF cross sections are almost the same for both the systems in the above barrier region, the suppression of σCF at above the barrier is less for the 7Li+64Ni system than for the 6+64Ni system. Also direct cluster transfer has been identified as the probable source for producing large enhancement in TF cross sections.

  16. 6Li foil thermal neutron detector

    SciTech Connect

    Ianakiev, Kiril D; Swinhoe, Martyn T; Favalli, Andrea; Chung, Kiwhan; Macarthur, Duncan W

    2010-01-01

    In this paper we report on the design of a multilayer thermal neutron detector based on {sup 6}Li reactive foil and thin film plastic scintillators. The {sup 6}Li foils have about twice the intrinsic efficiency of {sup 10}B films and about four times higher light output due to a unique combination of high energy of reaction particles, low self absorption, and low ionization density of tritons. The design configuration provides for double sided readout of the lithium foil resulting in a doubling of the efficiency relative to a classical reactive film detector and generating a pulse height distribution with a valley between neutron and gamma signals similar to {sup 3}He tubes. The tens of microns thickness of plastic scintillator limits the energy deposited by gamma rays, which provides the necessary neutron/gamma discrimination. We used MCNPX to model a multilayer Li foil detector design and compared it with the standard HLNCC-II (18 {sup 3}He tubes operated at 4 atm). The preliminary results of the {sup 6}Li configuration show higher efficiency and one third of the die-away time. These properties, combined with the very short dead time of the plastic scintillator, offer the potential of a very high performance detector.

  17. Challenges in describing nuclear reactions outcomes at near-barrier energies

    NASA Astrophysics Data System (ADS)

    Dasgupta, M.; Simpson, E. C.; Kalkal, S.; Cook, K. J.; Carter, I. P.; Hinde, D. J.; Luong, D. H.

    2017-01-01

    The properties of light nuclei such as 6Li, 7Li, 9Be and 12C, and their reaction outcomes are known to be strongly influenced by their underlying α-cluster structure. Reaction models do not yet exist to allow accurate predictions of outcomes following a collision of these nuclei with another nucleus. As a result, reaction models within GEANT, and nuclear fusion models do not accurately describe measured products or cross sections. Recent measurements at the Australian National University have shown new reaction modes that lead to breakup of 6Li, 7Li into lighter clusters, again presenting a further challenge to current models. The new observations and subsequent model developments will impact on accurate predictions of reaction outcomes of 12C - a three α-cluster nucleus – that is used in heavy ion therapy.

  18. Theoretical calculations and analysis for n + 6Li reaction

    NASA Astrophysics Data System (ADS)

    Tao, Xi; Wang, Jimin; Chen, Guochang; Shen, Qingbiao

    2017-09-01

    R-matrix theory is an important methodology for applications on light, medium and heavy mass nuclides nuclear reaction in the resonance energy range. Full R-matrix formalism contains the diagonal elements of the energy levels matrix and it is a rigorous theory. Because of different assumptions and approximations, many kinds of R-matrix derived methods are obtained. The new R-matrix code FDRR is presented and includes 4 kinds of R-matrix applications. It can be used for calculating integral cross sections and angular distributions of 2-bodies reactions. The cross sections and angular distributions of n+ 6Li reaction are calculated and analyzed by FDRR code. The results are in good agreement with experimental data below 20 MeV.

  19. Lithium and Isotopic Ratio Li6/Li7 in Magnetic roAp Stars as an Indicator of Active Processes

    NASA Astrophysics Data System (ADS)

    Polosukhina, N.; Shavrina, A.; Lyashko, D.; Nesvacil, N.; Drake, N.; Smirnova, M.

    2015-04-01

    The lines of lithium at 6708 Å and 6103 Å are analyzed in high resolution spectra of some sharp-lined and slowly rotating roAp stars. Three spectral synthesis codes— STARSP, ZEEMAN2, and SYNTHM—were used. New lines of rare earth elements (REE) from the DREAM database and the lines calculated on the basis of the NIST energy levels were included. Magnetic splitting and other line broadening processes were taken into account. For both lithium lines, the enhanced abundances of lithium in the atmospheres of the stars studied are obtained. The lithium abundance determined from the Li 6103 Å line is higher than that from the Li 6708 Å for all the stars. This may be evidence of vertical lithium stratification, abnormal temperature distribution, or unidentified blending of the 6103 Å line. Our work on two roAp stars, HD 83368 and HD 60435 (Shavrina et al. 2001) provides evidence of an enhanced lithium abundance near the magnetic-field poles. We can expect similar effects in the sharp-lined roAp stars. High lithium abundance for all the stars and the estimates of the 6Li/7Li ratio (0.2-0.5) can be explained by production of Li in the cosmic ray spallation reactions in the interstellar medium where the stars were born, and by preservation of the original 6Li and 7Li by strong magnetic fields of these stars. The values of the 6Li/7Li ratio expected from production by cosmic rays are about 0.5-0.8 (Knauth et al. 2003; Webber et al. 2002). New laboratory and theoretical gf-values for REE lines are necessary in order to refine our estimates of lithium abundances and the isotopic ratio.

  20. Ab initio calculation of 7Li photodisintegration

    NASA Astrophysics Data System (ADS)

    Bacca, Sonia; Arenhövel, Hartmuth; Barnea, Nir; Leidemann, Winfried; Orlandini, Giuseppina

    2004-12-01

    The 7Li total photoabsorption cross section is calculated microscopically, using the semi-realistic AV4' nucleon-nucleon potential. The interaction of the final 7-nucleon system is fully taken into account via the Lorentz integral transform (LIT) method. For the calculation of the LIT we use expansions in hyperspherical harmonics (HH) in conjunction with the HH effective interaction (EIHH) approach. The convergence of the LIT expansion is discussed in detail. The calculated cross section agrees quite well with the available experimental data, which cover an energy range from threshold up to 100 MeV.

  1. Diffusion of 6Li in Ta and W

    NASA Astrophysics Data System (ADS)

    Vacik, J.; Hnatowicz, V.; Köster, U.; Cervena, J.; Havranek, V.; Pasold, G.

    2006-08-01

    The objective of this work was the study of 6Li diffusion in the Ta and W refractory metals. The samples were prepared by ion implantation of 380 keV 6Li+ ions into W and Ta thin foils (up to the fluence of 1016 ions/cm2) and annealed up to the temperature 1940 °C. The depth profiles of 6Li were determined using the Thermal Neutron Depth Profiling (TNDP) technique. The results showed that diffusion of 6Li in both W and Ta foils is very complex and cannot be described by simple Fick's laws. Trapping centers (in the subsurface layers of both W and Ta metals) were supposed in a trial to explain the 6Li diffusion behaviour. However, the 6Li depth profiles were only partly explained. Other aspects are necessary to take into account for more proper quantification; such as spatially dependent diffusion coefficients, etc.

  2. Spectroscopic information of 6Li from elastic scattering of deuterons, 3He and 4He by 6Li

    NASA Astrophysics Data System (ADS)

    Amar, A.

    2014-07-01

    The elastic scattering of deuterons, 3He and 4He on 6Li at different incident energies have been analyzed in the framework of the optical model (OM) using ECIS88 as well as SPI GENOA codes. The optical potential parameters were extracted in the phenomenological treatment. A good agreement between theoretical and experimental differential cross-sections was obtained in whole angular range. Parameters for real part of potential have been also calculated microscopically with double-folding model for the d, 3He and 4He scattering, respectively, using DFPOT code. The elastic transfer mechanism has been studied by coupled reaction channel (CRC) method using FRESCO code. Spectroscopic amplitudes of 6Li ≡ t + 3He and 6Li ≡ α + d configurations have been extracted from d, 3He and 4He scattering on 6Li at wide energy range. A comparison between spectroscopic amplitudes obtained from deuteron and α elastically scattering from 6Li has been made. The extracted spectroscopic amplitudes of 6Li ≡ 4He + d(SF = SA2) from 6Li(d, 6Li)d and 6Li(α, 6Li)α are not the same as expected theoretically.

  3. Complete and incomplete fusion dynamics of 6,7Li + 159Tb reactions near the Coulomb barrier

    NASA Astrophysics Data System (ADS)

    Gautam, Manjeet Singh; Grover, Neha; Sharma, Manoj K.

    2017-01-01

    The complete fusion (CF) and incomplete fusion (ICF) cross-sections are estimated for 6, 7Li + 159Tb reactions using the energy-dependent Woods-Saxon potential model (EDWSP model) and dynamical cluster-decay model (DCM). The CF data of the 6Li + 159Tb(7Li + 159Tb) reaction at above barrier energies is suppressed with reference to expectations of the EDWSP model by 25% (20%) which is smaller than the reported data by ˜ 9% (6%). This suppression is correlated with the projectile breakup effect. The projectiles 6,7Li are loosely bound systems, which may break up into charged fragments prior to reaching the fusion barrier and subsequently one of the fragment is captured by the target leading to the suppression of fusion data at above barrier energies. The sum of CF and ICF, which is termed as total fusion cross-section (TF), removes the discrepancies between theoretical predictions and the above barrier complete fusion data and hence is adequately explained via the EDWSP model over a wide range of energy spread across the Coulomb barrier. In addition to fusion, the decay mechanism of 6Li + 159Tb reaction is studied within the framework of the dynamical cluster-decay model (DCM). The breakup of the projectile (6Li) in the entrance channel indicates the presence of ICF, which is investigated further using the collective clusterization approach of DCM. The present theoretical analysis suggests that a larger barrier modification is needed to address the fusion data of chosen reactions in the below barrier energy region.

  4. Four-time 7Li stimulated-echo spectroscopy for the study of dynamic heterogeneities: Application to lithium borate glass

    NASA Astrophysics Data System (ADS)

    Storek, M.; Tilly, J. F.; Jeffrey, K. R.; Böhmer, R.

    2017-09-01

    To study the nature of the nonexponential ionic hopping in solids a pulse sequence was developed that yields four-time stimulated-echo functions of previously inaccessible spin-3/2-nuclei such as 7Li. It exploits combined Zeeman and octupolar order as longitudinal carrier state. Higher-order correlation functions were successfully generated for natural-abundance and isotopically-enriched lithium diborate glasses. Four-time 7Li measurements are presented and compared with two-time correlation functions. The results are discussed with reference to approaches devised to quantify the degree of nonexponentiality in glass forming systems and evidence for the occurrence of dynamic heterogeneities and dynamic exchange were found. Additional experiments using the 6Li species illustrate the challenge posed by subensemble selection when the dipolar interactions are not very much smaller than the quadrupolar ones.

  5. Four-time (7)Li stimulated-echo spectroscopy for the study of dynamic heterogeneities: Application to lithium borate glass.

    PubMed

    Storek, M; Tilly, J F; Jeffrey, K R; Böhmer, R

    2017-09-01

    To study the nature of the nonexponential ionic hopping in solids a pulse sequence was developed that yields four-time stimulated-echo functions of previously inaccessible spin-3/2-nuclei such as (7)Li. It exploits combined Zeeman and octupolar order as longitudinal carrier state. Higher-order correlation functions were successfully generated for natural-abundance and isotopically-enriched lithium diborate glasses. Four-time (7)Li measurements are presented and compared with two-time correlation functions. The results are discussed with reference to approaches devised to quantify the degree of nonexponentiality in glass forming systems and evidence for the occurrence of dynamic heterogeneities and dynamic exchange were found. Additional experiments using the (6)Li species illustrate the challenge posed by subensemble selection when the dipolar interactions are not very much smaller than the quadrupolar ones. Copyright © 2017 Elsevier Inc. All rights reserved.

  6. A method for investigation of the D(4He, γ)6Li reaction in the Ultralow energy region under a high background

    NASA Astrophysics Data System (ADS)

    Bystritsky, V. M.; Dudkin, G. N.; Krylov, A. R.; Gazi, S.; Huran, J.; Nechaev, B. A.; Padalko, V. N.; Sadovsky, A. B.; Tuleushev, Yu. Zh.; Filipowicz, M.; Philippov, A. V.

    2016-07-01

    The cosmological lithium problem, that is, a noticeable discrepancy between the predicted and observed abundances of lithium, is in conflict with the Standard Big Bang Nucleosynthesis model. For example, the abundance of 7Li is 2-4 times smaller than predicted by the Standard Big Bang Nucleosynthesis. As to the abundance of 6Li, recent more accurate optical investigations have yielded only the upper limit on the 6Li/7Li ratio, which makes the problem of 6Li abundance and accordingly of disagreement with the Standard Big Bang Nucleosynthesis predictions less acute. However, experimental study of the D(4He, γ)6Li reaction cross section is still of current importance because there is a theoretical approach predicting its anomalously large value in the region of energies below the Standard Big Bang Nucleosynthesis energy. The work is dedicated to the measurement of the cross section for the D(4He, γ)6Li reaction proceeding in zirconium deuteride at the incident 4He+ion energy of 36 keV. The experiment is performed at a pulsed Hall plasma accelerator with an energy spread of 20% FWHM. A method for direct measurement of the background from the reaction chain D(4He, 4He)D→D(D, n)3He→(n, γ) and/or (n, n‧γ) ending with activation of the surrounding material by neutrons is proposed and implemented in the work. An upper limit on the D(4He, γ)6Li reaction cross section σ≤7·10-36 cm2 at the 90% confidence level is obtained.

  7. Breakup Reactions and Exclusive Measurements in the {sup 6,7}Li+{sup 144}Sm Systems

    SciTech Connect

    Heimann, D. Martinez; Pacheco, A. J.; Arazi, A.; Figueira, J. M.; Negri, A. E.; Capurro, O. A.; Carnelli, P.; Fimiani, L.; Grinberg, P.; Marti, G. V.; Testoni, J. E.; Monteiro, D. S.; Marta, H. D.

    2009-06-03

    The breakup of the projectile-like nuclei in reactions induced by 30 MeV {sup 6}Li and {sup 7}Li beams on a {sup 144}Sm target have been measured through the coincident detection of the in-plane emitted light particles. The primary ion that undergoes breakup has been identified and the physically meaningful variables that characterize the reaction have been obtained on a purely experimental basis. Distributions have been obtained for both the binary emission angle and for the breakup emission angle in the reference frame of the breakup products.

  8. Effect of breakup on elastic scattering for the {sup 6,7}Li+{sup 59}Co systems

    SciTech Connect

    Souza, F. A.; Leal, L. A. S.; Carlin, N.; Munhoz, M. G.; Neto, R. Liguori; Moura, M. M. de; Suaide, A. A. P.; Szanto, E. M.; Toledo, A. Szanto de; Takahashi, J.

    2007-04-15

    The elastic scattering for the {sup 6,7}Li+{sup 59}Co systems was investigated in the bombarding energy range 12 MeV{<=}E{sub lab}{<=}30 MeV by means of an analysis using the Sao Paulo potential, through which the behavior of the real and imaginary parts as function of the bombarding energy was established. The experimental results suggest that overall there is an evidence of the usual threshold anomaly for both systems, although for the {sup 6}Li+{sup 59}Co system, an evidence of the breakup threshold anomaly could also be questioned.

  9. Colorado School of Mines Low Energy Nuclear Physics Project technical progress report

    SciTech Connect

    Cecil, F.E.

    1990-01-05

    This report summarizes the activity and accomplishments of the Colorado School of Mines Low Energy Nuclear Physics project during the calendar year 1989. Many of the projects which were anticipated in the original grant proposal have been completed. Among these completed projects we include of study of the radiative capture of low energy protons on {sup 6}Li, {sup 7}Li, {sup 9}Be, and {sup 11}B. Preliminary measurements of the branching ratios and yields of these reactions were reported in last year's Technical Progress Report. These measurements are now complete and have been used to extract the respective astrophysical S-factors and the corresponding thermonuclear reactivities. While not complete, progress has been made in some of the other originally proposed studies. Among these include a fairly extensive study of the interaction of low energy deuterons with {sup 6}Li and {sup 7}Li. In the course of this study we have made a solid observation of the Oppenheimer-Phillips effect in the D-{sup 6}Li system. Progress has been made in our study of the radiative capture of alpha particles by deuterons, {sup 6}Li, and {sup 7}Li but considerable work remains in these studies. In our earlier reports we noted the observation of d-d reactions during the bombardment of deuterated targets with energetic beams of protons, alpha particles, and other light-to-medium ions. We believe we now understand this phenomenon and feel it has some fairly significant consequences both for our studies and for those of other researchers. Our susceptibility to mob hysteria led us to invest a significant effort in cold nuclear fusion, both employing a fairly unique accelerator based approach at CSM and as one of the gamma ray diagnosticians on the Princeton Plasma Physics Laboratory's Cold Fusion Task Force.

  10. Primordial α +d →6Li+γ reaction and second lithium puzzle

    NASA Astrophysics Data System (ADS)

    Mukhamedzhanov, A. M.; Shubhchintak, Bertulani, C. A.

    2016-04-01

    During the Big Bang, 6Li was synthesized via the 2H(α ,γ ) 6Li reaction. After almost 25 years of the failed attempts to measure the 2H(α ,γ ) 6Li reaction in the laboratory at Big Bang energies, just recently the LUNA Collaboration presented the first successful measurements at two different Big Bang energies [Anders et al., Phys. Rev. Lett. 113, 042501 (2014), 10.1103/PhysRevLett.113.042501]. In this paper we will discuss how to improve the accuracy of the direct experiment. To this end the photon's angular distribution is calculated in the potential model. It contains contributions from electric dipole and quadrupole transitions and their interference, which dramatically changes the photon's angular distribution. The calculated distributions at different Big Bang energies have a single peak at ˜50∘ . These calculations provide the best kinematic conditions to measure the 2H(α ,γ ) 6Li reaction. The expressions for the total cross section and astrophysical factor are also derived by integrating the differential cross section over the photon's solid angle. The LUNA data are in excellent agreement with our calculations using a potential approach combined with a well established asymptotic normalization coefficient for 6Li→α +d . Comparisons of the available experimental data for the S24 astrophysical factor and different calculations are presented. The Big Bang lithium isotopic ratio 6Li/7Li=(1.5 ±0.3 ) ×10-5 following from the LUNA data and the present analysis are discussed in the context of the disagreement between the observational data and the standard Big Bang model, which constitutes the second

  11. {alpha} resonance structure in {sup 11}B studied via resonant scattering of {sup 7}Li+{alpha}

    SciTech Connect

    Yamaguchi, H.; Hashimoto, T.; Hayakawa, S.; Binh, D. N.; Kahl, D.; Kubono, S.; Wakabayashi, Y.; Kawabata, T.; Teranishi, T.

    2011-03-15

    A new measurement of {alpha} resonant scattering on {sup 7}Li was performed over the excitation energy of 10.2-13.0 MeV in {sup 11}B at the low-energy RI beam facility CNS Radioactive Ion Beam separator (CRIB) of the Center for Nuclear Study (CNS), University of Tokyo. The excitation function of {sup 7}Li+{alpha} at 180 deg. in the center-of-mass system was successfully measured for the first time with the inverse kinematics method, providing important information on the {alpha} cluster structure in {sup 11}B and the reaction rate of {sup 7}Li({alpha},{gamma}), which is relevant to the {sup 11}B production in the {nu} process in core-collapse supernovae. The excitation function of the {sup 7}Li({alpha},p) reaction cross section for 11.7-13.1 MeV was also measured.

  12. Exclusive Measurements of Breakup Reactions in the {sup 7}Li+{sup 144}Sm System

    SciTech Connect

    Heimann, D. Martinez; Pacheco, A. J.; Arazi, A.; Figueira, J. M.; Negri, A.; Capurro, O. A.; Carnelli, P.; Fimiani, L.; Grinberg, P.; Marti, G. V.; Testoni, J. E.; Monteiro, D. S.; Marta, H. D.

    2009-03-04

    Breakup reactions induced by a 30 MeV {sup 7}Li beam on a {sup 144}Sm target were measured through the coincident detection of the light particles emitted in the reaction plane. The emphasis of the measurements and data analysis was placed in the complete characterization of the reaction by means of the identification of the breakup products and the experimental extraction of the physically relevant magnitudes. The coincident yield of the emitted light particles was compared with the results of kinematical calculations that were done assuming different distributions for these magnitudes and taking into account the geometric response of the detection system. The results of this comparison indicate in all cases a clear dominance of a process compatible with the breakup of {sup 6}Li through the 3{sup +} resonant state at 2.186 MeV following one-neutron transfer from the projectile to the target, over the breakup of the projectile itself. Relative cross sections as a function of the emission angle of the {sup 6}Li and the in-plane anisotropy of the subsequent emission of breakup products were extracted from the data.

  13. Elastic and inelastic scattering of 15N ions by 7Li at 81 MeV versus that of 14N ions by 7Li at 80 and 110 MeV

    NASA Astrophysics Data System (ADS)

    Rudchik, A. T.; Rudchik, A. A.; Muravynets, L. M.; Kemper, K. W.; Rusek, K.; Piasecki, E.; Trzcińska, A.; Koshchy, E. I.; Pirnak, Val. M.; Ponkratenko, O. A.; Strojek, I.; Stolarz, A.; Herashchenko, O. V.; Stepanenko, Yu. M.; Plujko, V. A.; Sakuta, S. B.; Siudak, R.; Szczurek, A.

    2017-02-01

    Angular distributions of the elastic and inelastic scattering of 15N ions by 7Li nuclei were measured at the energy Elab (15N) = 81 MeV (Ec.m. = 25.77 MeV). The data were analyzed within the coupled-reaction-channels method. The elastic and inelastic scattering, spin reorientations of 7Li as well as the more important one- and two-step transfer reactions were included in the channels-coupling scheme. The parameters of 7Li +15N optical potential of Woods-Saxon form as well as deformation parameters of these nuclei were deduced. The analysis showed that the forward angle elastic scattering is dominated by pure potential scattering whereas the middle and large angle scattering gets a contribution from the ground state reorientation of 7Li. Contributions from particle transfers were negligible for the present scattering system. The 7Li +15N elastic scattering was compared with that of 7Li +14N at the energies Elab (14N) = 80 MeV and 110 MeV. Different contributions to the elastic scatterings from other nuclear processes are shown to be responsible for the isotopic difference observed in the large angle scattering.

  14. New nuclear physics for big bang nucleosynthesis

    SciTech Connect

    Boyd, Richard N.; Brune, Carl R.; Fuller, George M.; Smith, Christel J.

    2010-11-15

    We discuss nuclear reactions which could play a role in big bang nucleosynthesis. Most of these reactions involve lithium and beryllium isotopes and the rates for some of these have not previously been included in BBN calculations. Few of these reactions are well studied in the laboratory. We also discuss novel effects in these reactions, including thermal population of nuclear target states, resonant enhancement, and nonthermal neutron reaction products. We perform sensitivity studies which show that even given considerable nuclear physics uncertainties, most of these nuclear reactions have minimal leverage on the standard BBN abundance yields of {sup 6}Li and {sup 7}Li. Although a few have the potential to alter the yields significantly, we argue that this is unlikely.

  15. Search for P-odd asymmetry in the. cap alpha. emission in the capture of polarized thermal neutrons by /sup 6/Li and /sup 10/B nuclei

    SciTech Connect

    Vesna, V.A.; Egorov, A.I.; Kolomenskii, A.; Kornyushkin, A.F.; Lobashev, V.M.; Okunev, I.S.; Peskov, B.G.; Pirozhkov, A.N.; Smotritskii, L.M.; Titov, N.A.

    1983-09-10

    Measurements by an integral method in a geometry ruling out an effect of a P-even left-right asymmetry have yielded limitations on the magnitude of the P-odd asymmetry in several reactions: Vertical Bara/sub p/Vertical Bar<1.4 x 10/sup -6/ for the reaction /sup 6/Li(n,..cap alpha..)/sup 3/H, Vertical Bara/sub p/Vertical Bar<8 x 10/sup -6/ for the reaction /sup 10/B(n,..cap alpha../sub 0/)/sup 7/Li, and Vertical Bara/sub p/Vertical Bar<1.5 x 10/sup -6/ for the reaction /sup 10/B(n,..cap alpha../sub 1/)/sup 7/Li* (90% confidence level).

  16. Li-6/Li-7, B-10/B-11, and Li-7/B-11/Si-28 individual IDPs

    NASA Technical Reports Server (NTRS)

    Xu, Y.-L.; Song, L.-G.; Zhang, Y.-X.; Fan, C.-Y.

    1994-01-01

    At the initial stage of the development of our solar system, the solar nebula is presumably composed of H-1, H-2, He-3, He-4, and Li-7, which were made during the Big Band, and C, N, O, . . ., which are products of nearby supernova explosions. Li-6 nuclei (together with about equal amounts of Li-7), Be-9, B-10, and B-11 were produced later by cosmic ray particles bombarding the local interstellar C, N, O, . . . nuclei before the nebula condensed to become the Sun and the planets. Thus, the ratio Li-6/Li-7 is a measure of the length of the early epoch of the solar system. In this paper we shall report the measurement of Li-7/Li-6, B-11/B-10, and Li-7/B-11/Si-28 of four IDP's obtained from Johnson Space Center and discuss the findings.

  17. Differential cross section measurements for the 6Li(n,t)alpha reaction in the few MeV region

    SciTech Connect

    Devlin, Matthew J; Taddeucci, Terence N; Hale, Gerald M; Haight, Robert C; O' Donnell, Johhn M

    2008-01-01

    New measured differential cross sections of tritons and alpha particles following the {sup 6}Li(n,t){alpha} reaction are reported for incident neutron energies between 0.2 and approximately 20 MeV. The neutrons were produced by spallation at the WNR facility at the Los Alamos Neutron Science CEnter (LANSCE), with the incident neutron energy determined by the time-of-flight method. Four E-{Delta}E telescopes were used at eight laboratory angles. These data have been incorporated into a prior R-matrix fit for the compound {sup 7}Li system, and result in an (n,t) reaction cross section that is 4% to 10% higher than previous evaluations in the 1-3 MeV incident neutron energy region.

  18. Near- and subbarrier elastic and quasielastic scattering of the weakly bound {sup 6}Li projectile on {sup 144}Sm

    SciTech Connect

    Monteiro, D. S.; Otomar, D. R.; Lubian, J.; Gomes, P. R. S.; Arazi, A.; Figueira, J. M.; Heimann, D. Martinez; Negri, A. E.; Pacheco, A. J.; Niello, J. O. Fernandez; Guimaraes, V.

    2009-01-15

    High-precision data of backward-angle elastic and quasielastic scattering for the weakly bound {sup 6}Li projectile on {sup 144}Sm target at deep-sub-barrier, near-, and above-barrier energies were measured. From the deep-sub-barrier data, the surface diffuseness of the nuclear interacting potential was studied. Barrier distributions were extracted from the first derivatives of the elastic and quasielastic excitation functions. It is shown that sequential breakup through the first resonant state of the {sup 6}Li is an important channel to be included in coupled-channels calculations, even at deep-sub-barrier energies.

  19. Reaction mechanisms in the 6Li+ 52Cr system

    NASA Astrophysics Data System (ADS)

    Pandey, Bhawna; Prajapati, P. M.; Patel, D.; Desai, V. V.; Kumar, H.; Suranarayana, S. V.; Nayak, B. K.; Saxena, Alok; Jakhar, S.; Rao, CVS; Basu, T. K.

    2015-01-01

    Reactions induced by the weakly bound 6Li projectile interacting with the intermediate mass target 52Cr are investigated. The choice of this particular reaction in our study is because it is proposed as a surrogate reaction [6Li(52Cr, d)56Fe*] for the measurement of 55Fe(n,p) reaction cross-section, which has been found to be very important in fusion reactor studies. All the conditions which have to be satisfied for using the surrogate method have been checked. The energy of 6Li beam is selected in a way so as to get equivalent neutron energy in the region of 9-14 MeV, which is of primary interest in fusion reactor application. In the present work, statistical model calculations PACE (Projection-Angular-Momentum-Coupled-Evaporation), ALICE and Continuum-Discretized-Coupled-Channel (CDCC: FRESCO) have been used to provide information for the 6Li + 52Cr system and the respective contributions of different reaction mechanisms. The present theoretical work is an important step in the direction towards studying the cross-section of the 55Fe(n, p)55Mn reaction by surrogate method.

  20. Investigations of 6LiIn1-xGaxSe2 semi-insulating crystals for neutron detection

    NASA Astrophysics Data System (ADS)

    Wiggins, Brenden; Bell, Joseph; Burger, Arnold; Stassun, Keivan; Stowe, Ashley C.

    2015-08-01

    Neutron detectors are used for illicit material detection, neutron radiography, stellar investigations of chemical content including biological compounds in planetary terrain and to monitor nuclear power plant fuel products and radioactive waste. Li-containing chalcogenide materials are promising alternative thermal neutron detection materials due to the incorporation of the 6Li isotope at high density. 6LiInSe2 is limited in its effective thermal neutron efficiency by 115In neutron capture which results in gamma decay rather than charge creation. This study includes investigations of mixed crystalline material 6LiIn1-xGaxSe2 where the indium concentration is reduced by Ga substitution. The optical properties have been tuned by gallium substitution and radiation response has been observed.

  1. Method for determining fast-alpha-particle confinement in tokamak plasmas using resonant nuclear reactors

    SciTech Connect

    Cecil, F.E.; Zweben, S.J.; Medley, S.S.

    1986-03-01

    The resonant nuclear reactions D(..cap alpha..,..gamma..)/sup 6/Li, /sup 6/Li(..cap alpha..,..gamma..)/sup 10/B, and /sup 7/Li(..cap alpha..,..gamma..)/sup 11/B are examined as diagnostics of fast-alpha-particle confinement in tokamak plasmas. Gamma rays from these resonant reactions with energies from 2.1 MeV to 9.2 MeV may be used to infer the alpha-particle population between energies of 0.4 MeV and 2.6 MeV. The ratio of these alpha-burnup reactions to the reactions T(D,..gamma..)/sup 5/He and /sup 3/He(D,..gamma..)/sup 5/Li provides a technique for the measurement of alpha confinement.

  2. Trials for the cosmological 7Li problem with 7Be beams at CRIB and collaborating studies

    NASA Astrophysics Data System (ADS)

    Hayakawa, S.

    2017-09-01

    For many years, the cosmological ^7 Li problem has been tackled from various aspects. The nuclear reaction data have also been improved, but still there remains some ambiguities. We review our experimental plans to measure the cross sections of three key reactions which act to destroy ^7 Be during the Big-Bang Nucleosynthesis (BBN). These experiments are all based on ^7 Be beams produced at Center-for-Nuclear-Study Radioactive Ion Beam separator (CRIB) in collaborations mainly with research groups from INFN-LNS and RCNP. The preliminary result of the previous experiment and the future plan are discussed.

  3. Coulomb breakup of 6Li into α+d in the field of a 208Pb ion

    NASA Astrophysics Data System (ADS)

    Irgaziev, B. F.; Nabi, Jameel-Un; Khan, Darwaish

    2011-12-01

    The triple differential cross section of the 208Pb(6Li,αd)208Pb quasielastic breakup is calculated at a collision energy of 156 MeV and a scattering angle range of 2∘-6∘. We fit the parameters of the Woods-Saxon potential using the experimental α-d phase shifts for different states to describe the relative motion of the α particle and deuteron. To check the validity of the two particle approach for the α-d system, we apply a potential model to describe the 2H(α,γ)6Li radiative capture. We calculate the Coulomb breakup using the semiclassical method while an estimation of the nuclear breakup is made on the basis of the diffraction theory. A comparison of our calculation with the experimental data of Kiener [Phys. Rev. CPRVCAN0556-281310.1103/PhysRevC.44.2195 44, 2195 (1991)] gives evidence for the dominance of the Coulomb dissociation mechanism and the contribution of nuclear distortion, but is essentially smaller than the value reported by Hammache [Phys. Rev. CPRVCAN0556-281310.1103/PhysRevC.82.065803 82, 065803 (2010)]. The results of our calculation for the triple cross sections (contributed by the Coulomb and nuclear mechanisms) of the 6Li breakup hint toward a forward-backward asymmetry in the relative direction of the α particle and deuteron emission, especially at smaller scattering angles, in the 6Li center-of-mass (c.m.) system.

  4. An update on the big bang nucleosynthesis prediction for {sup 7}Li: the problem worsens

    SciTech Connect

    Cyburt, Richard H; Fields, Brian D; Olive, Keith A E-mail: bdfields@uiuc.edu

    2008-11-15

    The lithium problem arises from the significant discrepancy between the primordial {sup 7}Li abundance as predicted by big bang nucleosynthesis (BBN) theory and the Wilkinson Microwave Anisotropy Probe (WMAP) baryon density, and the pre-Galactic lithium abundance inferred from observations of metal-poor (Population II) stars. This problem has loomed for the past decade, with a persistent discrepancy of a factor of 2-3 in {sup 7}Li/H. Recent developments have sharpened all aspects of the Li problem. Namely: (1) BBN theory predictions have sharpened due to new nuclear data; in particular, the uncertainty on the reaction rate for{sup 3}He({alpha},{gamma}){sup 7}Be has reduced to 7.4%, nearly a factor of 2 tighter than previous determinations. (2) The WMAP five-year data set now yields a cosmic baryon density with an uncertainty reduced to 2.7%. (3) Observations of metal-poor stars have tested for systematic effects. With these, we now find that the BBN+WMAP predicts{sup 7}Li/H = (5.24{sub -0.67}{sup +0.71}) Multiplication-Sign 10{sup -10}. The central value represents an increase by 23%, most of which is due to the upward shift in the{sup 3}He({alpha},{gamma}){sup 7}Be rate. More significant is the reduction in the{sup 7}Li/H uncertainty by almost a factor of 2, tracking the reduction in the{sup 3}He({alpha},{gamma}){sup 7}Be error bar. These changes exacerbate the Li problem; the discrepancy is now a factor 2.4 or 4.2{sigma} (from globular cluster stars) to 4.3 or 5.3{sigma} (from halo field stars). Possible resolutions to the lithium problem are briefly reviewed, and key experimental and astronomical measurements highlighted.

  5. Role of Barrier Modification and Nuclear Structure Effects in Sub-Barrier Fusion Dynamics of Various Heavy Ion Fusion Reactions

    NASA Astrophysics Data System (ADS)

    Gautam, Manjeet Singh; Vinod, K.; Kumar, Hitender

    2017-10-01

    The role of barrier modifications and the relevant nuclear structure effects in the fusion of the {}_8{}^{16}O+{}_{62}{}^{144,148,150,152,154}Sm and {}_3{}^{6,7}Li+{}_{62}{}^{152}Sm systems is analyzed within the context of the energy-dependent Woods-Saxon potential model (EDWSP model) and the coupled channel model. For the {}_8{}^{16}O+{}_{62}{}^{144,148,150,152,154}Sm reactions, where the colliding pairs are stable against breakup, the collective excitations and/or static deformations are sufficient to account for the observed fusion enhancement. In contrast, the model calculations overpredict the complete fusion data at above - barrier energies for the {}_3{}^{6,7}Li+{}_{62}{}^{152}Sm systems, where the importance of projectile breakup effects has been pointed out. Due to the low threshold of the alpha-breakup channel, the weakly bound projectiles ({}_3{}^{6,7}Li) break up into charged fragments before reaching the fusion barrier and consequently the complete fusion cross section is suppressed by 28% (25%) in the {}_3{}^6Li+{}_{62}{}^{152}Sm({}_3{}^7Li+{}_{62}{}^{152}Sm) reaction with respect to predictions of coupled channel calculations. However, the EDWSP model based calculations can minimize the suppression factor by as much as of 13% (8%) in the {}_3{}^6Li+{}_{62}{}^{152}Sm({}_3{}^7Li+{}_{62}{}^{152}Sm) reaction with reference to the predictions made by the coupled channel calculations. Therefore, the complete fusion data of the {}_3{}^6Li+{}_{62}{}^{152}Sm({}_3{}^7Li+{}_{62}{}^{152}Sm) reaction at above - barrier energies is reduced by 15% (17%) with respect to the expectations of the EDWSP model. The extracted suppression factors for the studied reactions are due to the modifications of the barrier profile as a consequence of the energy - dependence in nucleus-nucleus potential, and thus greater barrier modifications occur for more weakly bound system, which in turn, confirms the breakup of projectile in the incoming channel.

  6. The influence of temperature and salinity on the Li/Ca and d7Li of inorganic and biogenic carbonates

    NASA Astrophysics Data System (ADS)

    Marriott, C.; Staubwasser, M.; Crompton, R.; Henderson, G.

    2003-04-01

    Lithium is the sixth most abundant metal in the ocean. It is conservative with a residence time of around 1Ma and has two stable isotopes ^7Li and ^6Li that are not actively involved in biological processes. Isotopic fractionation is observed during incorporation into calcium carbonate but no previous work has systematically examined the controls on this fractionation. We have investigated Li incorporation and isotopic fraction in both inorganically precipitated calcite and coralline aragonite (1). In both cases there is an inverse correlation of Li concentration with temperature and no significant variation in isotopic fractionation. A decrease in D Li/Ca from 0.0092 to 0.0030 is seen over a temperature range of 5--30^oC, whilst an offset of approximately -8.5 ppm is seen in the δ^7Li ratio relative to the growth solution. The temperature dependence of Li/Ca has an increased sensitivity at low temperatures and might therefore be useful in examining changes in bottom water temperature. We are now investigating Li/Ca and δ^7Li of foraminifera. Previous work (2) has suggested little variability in Li/Ca with temperature, although this was for samples from warmer water where Li/Ca is not sensitive. In this study, Uvigerina are examined in a series of core top samples from the Arabian Sea with a depth range of 95--1800m and corresponding temperature range of 5--20^oC. A series of inorganic calcite samples have also been precipitated in order to examine the effect of salinity on Li/Ca, δ^7Li and δ44Ca over a salinity range of 10--50 psu. The distribution coefficient of Li shows a positive correlation with salinity over this range. δ^7Li and δ44Ca measurements for these samples are presently being analysed. (1) Marriott et al., 2002, GCA, 66, A485 (2) Delaney et al., 1985, GCA, 49, 1327

  7. Barrier distributions for the 7Li+27Al reaction

    NASA Astrophysics Data System (ADS)

    Cárdenas, W. H. Z.

    2010-08-01

    Barrier distributions can be obtained from the first derivative of the elastic and quasielastic (QEL) backward angle excitation functions [1]. In this work we present a study of the barrier distribution for the 7Li+27Al reaction from a Coupled-Channels Born Approximation (CCBA) calculations using the code FRESCO [2].

  8. Systematic description of the {sup 6}Li(n,n{sup '}){sup 6}Li{sup *}{yields}d+{alpha} reactions with the microscopic coupled-channels method

    SciTech Connect

    Matsumoto, T.; Ichinkhorloo, D.; Kato, K.; Hirabayashi, Y.; Chiba, S.

    2011-06-15

    We investigate {sup 6}Li(n,n{sup '}){sup 6}Li{sup *}{yields}d+{alpha} reactions by using the continuum-discretized coupled-channels method with the complex Jeukenne-Lejeune-Mahaux effective nucleon-nucleon interaction. In this study, the {sup 6}Li nucleus is described by a d+{alpha} cluster model. The calculated elastic cross sections for incident energies between 7.47 and 24.0 MeV are in good agreement with experimental data. Furthermore, we show that the neutron spectra for {sup 6}Li breakup states measured at selected angular points and incident energies can be also reproduced systematically.

  9. Population of Nuclei Via 7Li-Induced Binary Reactions

    SciTech Connect

    Clark, R M; Phair, L W; Descovich, M; Cromaz, M; Deleplanque, M A; Fallon, P; Lee, I Y; Macchiavelli, A O; McMahan, M A; Moretto, L G; Rodriguez-Vieitez, E; Sinha, S; Stephens, F S; Ward, D; Wiedeking, M; Bernstein, L A; Burke, J T; Church, J A

    2005-08-09

    The authors have investigated the population of nuclei formed in binary reactions involving {sup 7}Li beams on targets of {sup 160}Gd and {sup 184}W. The {sup 7}Li + {sup 184}W data were taken in the first experiment using the LIBERACE Ge-array in combination with the STARS Si {Delta}E-E telescope system at the 88-Inch Cyclotron of the Lawrence Berkeley National Laboratory. By using the Wilczynski binary transfer model, in combination with a standard evaporation model, they are able to reproduce the experimental results. This is a useful method for predicting the population of neutron-rich heavy nuclei formed in binary reactions involving beams of weakly bound nuclei and will be of use in future spectroscopic studies.

  10. Population of Nuclei Via 7Li-Induced Binary Reactions

    SciTech Connect

    Clark, Rodney M.; Phair, Larry W.; Descovich, M.; Cromaz, Mario; Deleplanque, M.A.; Fall on, Paul; Lee, I-Yang; Macchiavelli, A.O.; McMahan, Margaret A.; Moretto, Luciano G.; Rodriguez-Vieitez, E.; Sinha,Shrabani; Stephens, Frank S.; Ward, David; Wiedeking, Mathis

    2005-08-08

    The authors have investigated the population of nuclei formed in binary reactions involving {sup 7}Li beams on targets of {sup 160}Gd and {sup 184}W. The {sup 7}Li + {sup 184}W data were taken in the first experiment using the LIBERACE Ge-array in combination with the STARS Si {Delta}E-E telescope system at the 88-Inch Cyclotron of the Lawrence Berkeley National Laboratory. By using the Wilczynski binary transfer model, in combination with a standard evaporation model, they are able to reproduce the experimental results. This is a useful method for predicting the population of neutron-rich heavy nuclei formed in binary reactions involving beams of weakly bound nuclei formed in binary reactions involving beams of weakly bound nuclei and will be of use in future spectroscopic studies.

  11. Ab initio no-core solutions for 6Li

    NASA Astrophysics Data System (ADS)

    Shin, Ik Jae; Kim, Youngman; Maris, Pieter; Vary, James P.; Forssén, Christian; Rotureau, Jimmy; Michel, Nicolas

    2017-07-01

    We solve for properties of 6Li in the ab initio no-core full configuration (NCFC) approach and we separately solve for its ground state and {J}π ={2}2+ resonance with the Gamow shell model (GSM) in the Berggren basis. We employ both the JISP16 and chiral {{NNLO}}{opt} realistic nucleon-nucleon interactions and investigate the ground state energy, excitation energies, point proton root mean square (rms) radius and a suite of electroweak observables. We also extend and test methods to extrapolate the ground state energy, point proton rms radius, and electric quadrupole moment. We attain improved estimates of these observables in the NCFC approach by using basis spaces up through {N}\\max =18 that enable more definitive comparisons with experiment. Using the density matrix renormalization group approach with the JISP16 interaction, we find that we can significantly improve the convergence of the GSM treatment of the 6Li ground state and {J}π ={2}2+ resonance by adopting a natural orbital single-particle basis.

  12. Optimization of {sup 6}LiF:ZnS(Ag) Scintillator Light Yield Using Geant4

    SciTech Connect

    Yehuda-Zada, Y.; Pritchard, K.; Ziegler, J.B.; Cooksey, C.; Siebein, K.; Jackson, M.; Hurlbut, C.; Kadmon, Y.; Cohen, Y.; Maliszewskyj, N.C.; Ibberson, R.M.; Majkrzak, C.F.; Orion, Y.; Osovizky, A.

    2015-07-01

    Neutrons provide an effective tool to probe materials structure. Neutron diffraction is a method to determine the atomic and magnetic structure of a material based on neutron scattering. By this method a collimated incident beam of thermal neutrons heat the examined sample and based on the obtained diffraction pattern information on the structure of the material is provided. Research for developing a novel cold neutron detector for Chromatic Analysis Neutron Diffractometer Or Reflectometer (CANDOR) is underway at the NIST center for neutron research. The system unique design is aimed to provide over ten times fold faster analysis of materials than conventional system. In order to achieve the fast analysis a large number of neutron detectors is required. A key design constraint for this detector is the thickness of the neutron sensitive element. This is met using {sup 6}LiF:ZnS(Ag) scintillation material with embedded wavelength shifting (WLS) fibers conducting scintillation light to silicon photomultiplier photo-sensors. The detector sensitivity is determined by both the neutron capture probability ({sup 6}Li density) and the detectable light output produced by the ZnS(Ag) ionization, the latter of which is hindered by the fluorescence absorption of the scintillation light by the ZnS. Tradeoffs between the neutron capture probability, stimulated light production and light attenuation for determining the optimal stoichiometry of the {sup 6}LiF and ZnS(Ag) as well as the volume ratio of scintillator and fiber. Simulations performed using the GEANT4 Monte Carlo package were made in order to optimize the detector design. GEANT4 enables the investigation of the neutron interaction with the detector, the ionization process and the light transfer process following the nuclear process. The series of conversions required for this detector were modelled: - A cold neutron enters the sensor and is captured by {sup 6}Li in the scintillator mixture ({sup 6}Li (n,α) {sup 3}H

  13. Note: {sup 6}Li III light intensity observation for {sup 6}Li{sup 3+} ion beam operation at Hyper-Electron Cyclotron Resonance ion source

    SciTech Connect

    Muto, Hideshi; Ohshiro, Yukimitsu; Yamaka, Shoichi; Yamaguchi, Hidetoshi; Shimoura, Susumu; Watanabe, Shin-ichi; Oyaizu, Michihiro; Kobayashi, Kiyoshi; Kotaka, Yasuteru; Nishimura, Makoto; Kase, Masayuki; Kubono, Shigeru; Hattori, Toshiyuki

    2014-12-15

    The light intensity of {sup 6}Li III line spectrum at λ = 516.7 nm was observed during {sup 6}Li{sup 3+} beam tuning at the Hyper-Electron Cyclotron Resonance (ECR) ion source. Separation of ion species of the same charge to mass ratio with an electromagnetic mass analyzer is known to be an exceptionally complex process. However, {sup 6}Li III line intensity observation conducted in this study gives new insights into its simplification of this process. The light intensity of {sup 6}Li III line spectrum from the ECR plasma was found to have a strong correlation with the extracted {sup 6}Li{sup 3+} beam intensity from the RIKEN Azimuthal Varying Field cyclotron.

  14. Studies of 6Li-NMR properties in different salt solutions in low magnetic fields

    NASA Astrophysics Data System (ADS)

    Gordji-Nejad, A.; Colell, J.; Glöggler, S.; Blümich, B.; Appelt, S.

    2012-01-01

    In this article we report the longitudinal relaxation times ( T1) of various 6Li salts ( 6LiI, 6LiCl and 6LiNO 3) in D 2O and H 2O, measured in low magnetic fields ( B0 = 3.5 mT). This investigation serves the purpose of clarifying the relaxation behavior of different 6Li solutions and different concentrations. The measurement were undertaken to establish a framework for future applications of hyperpolarized 6Li in medical imaging, biological studies and investigations of lithium ion batteries. Time will pass during the transport of hyperpolarized lithium ions to the sample, which leads to a polarization loss. In order to store polarization as long as possible, it is necessary to examine which 6Li salt solution has the longest relaxation time T1. Longitudinal relaxation times of 6Li salts in D 2O and H 2O were investigated as a function of concentration and the most extended T1 was found for 6LiI in D 2O and H 2O. In agreement with the theory the relaxation time T1 of all 6Li salts increase with decreasing concentration. In the case of 6LiI in H 2O an inverse behavior was observed. We assume that the prolonged T1 times occur due to formation of 6LiOH upon the solution of 6LiI in H 2O, which settles as a precipitate. By diluting the solution, the precipitate continuously dissolves and approaches T1 of 6LiOH ( T1 ˜ 28 s), leading to a shorter T1 relaxation time.

  15. Efimov Physics in a 6Li-133Cs Atomic Mixture

    NASA Astrophysics Data System (ADS)

    Johansen, Jacob; Feng, Lei; Parker, Colin; Chin, Cheng; Wang, Yujun

    2015-05-01

    We investigate Efimov physics based on three-body recombination in an atomic mixture of 6Li and 133Cs in the vicinity of interspecies Feshbach resonances at 843 and 889 G. This allows us to compare the loss spectra near different resonances and test the universality of Efimov states. Theoretically the Efimov spectrum near 889 G is expected to be similar to that near 843 G, except that the first resonance is absent near the former Feshbach resonance. This is due to the difference in the Cs-Cs scattering length near the two resonances: At 843 G it is negative, whereas at 889 G it is positive. Although it is primarily the Li-Cs interactions that lead to Efimov resonances, the Cs-Cs scattering length is expected to influence the spectrum. This work is supported by NSF and Chicago MRSEC.

  16. Experimental Progress in a 6Li-133Cs Atomic Mixture

    NASA Astrophysics Data System (ADS)

    Feng, Lei; Johansen, Jacob; Parker, Colin; Chin, Cheng

    2015-05-01

    We report experimental progress in a mixture of 6Li and 133Cs. The mass imbalance of this system results in a particular challenge, as gravity has a significant influence on Cs position, but not on Li, separating the two gases at temperatures on the order of 200 nK. We overcome this difficulty using a two color optical dipole trap. We demonstrate mixing of these species below 100 nK in preparation for studies of quantum degenerate mixtures of this system. We further report on progress toward degeneracy and many-body physics measurements in this trap. Finally, we consider Efimov physics in this system, studying the effects of Cs-Cs interaction on the spectrum of LiCsCs trimers by a comparison of Feshbach resonances at 843 and 889 G. This work is supported by NSF and Chicago MRSEC.

  17. Colorado School of Mines low energy nuclear physics project. Final technical progress report

    SciTech Connect

    Cecil, F.E.

    1993-11-23

    This report summarizes the accomplishments of the project ``Studies of nuclear reactions at very low energies``. This project was undertaken in 1987 and completed in 1993. All but one of the major objectives of this study have been accomplished. Specifically the authors have completed their investigation of the (p,{gamma}) on light nuclei, a study of the Oppenheimer-Phillips effect, a measurements of the astrophysically interesting reaction D({alpha},{gamma}){sup 6}Li at low energies and an extension of the reaction D(d,{gamma}){sup 4}He to lower energies than previously observed. Preliminary investigation of te reaction {sup 7}Li({sup 3}He,p){sup 9}Be was begun and is continuing under a separate DOE grant. In addition to these tasks, they have completed some very interesting projects which were not included in the original proposal. These include a study of the (d,{gamma}) reactions on {sup 6}Li, {sup 7}Li and {sup 10}B and an investigation of the possibility of observing terrestrial antineutrinos from the beta decay chains of U and Th as a diagnostic of terrestrial heat flow.

  18. Records for conversion of laser energy to nuclear energy in exploding nanostructures

    NASA Astrophysics Data System (ADS)

    Jortner, Joshua; Last, Isidore

    2017-09-01

    Table-top nuclear fusion reactions in the chemical physics laboratory can be driven by high-energy dynamics of Coulomb exploding, multicharged, deuterium containing nanostructures generated by ultraintense, femtosecond, near-infrared laser pulses. Theoretical-computational studies of table-top laser-driven nuclear fusion of high-energy (up to 15 MeV) deuterons with 7Li, 6Li and D nuclei demonstrate the attainment of high fusion yields within a source-target reaction design, which constitutes the highest table-top fusion efficiencies obtained up to date. The conversion efficiency of laser energy to nuclear energy (0.1-1.0%) for table-top fusion is comparable to that for DT fusion currently accomplished for 'big science' inertial fusion setups.

  19. The Underground Nuclear Astrophysics in the Precision Era of BBN: Present Results and Future Perspectives

    NASA Astrophysics Data System (ADS)

    Gustavino, C.

    2016-01-01

    The abundance of light isotopes such as D, 3He, 4He, 6Li and 7Li produced during Big Bang Nucleosynthesis (BBN) only depends on particle physics, baryon density and relevant nuclear processes. At BBN energies (0.01 ÷ 1 MeV) the cross section of many BBN processes is very low because of the Coulomb repulsion between the interacting nuclei. As low-energy measurements on earth's surface are predominantly hampered by the effects of cosmic rays in the detectors, it is convenient to study the relevant reactions with facilities operating deep underground. Starting from the present uncertainty of the relevant parameters in BBN (i.e. baryon density, observed abundance of isotopes and nuclear cross-sections), it will be shown that the study of several reactions of the BBN chain, with existing or proposed underground accelerator facilities, can improve the accuracy of BBN calculations, providing a powerful tool to constrain astrophysics, cosmology and particle physics. In particular, a precise measurement of D(p, γ)3He reaction at BBN energies is of primary importance to calculate the baryon density of universe with an accuracy similar to the one obtained by Cosmic Microwave Background (CMB) experiments, and to constrain the number of active neutrino species. For what concern the so called ’’Lithium problems”, i.e. the disagreement between computed and observed abundances of the 7Li and 6Li isotopes, it will be also shown the importance of a renewed study of the D(α, γ) 6Li reaction.

  20. Marrying ab initio calculations and Halo-EFT: 7Li and 7Be radiative nucleon captures

    NASA Astrophysics Data System (ADS)

    Zhang, Xilin; Nollett, Kenneth; Phillips, Daniel

    2013-10-01

    We combine ab initio quantum-Monte-Carlo (QMC) calculations with the Halo-Effective-Field-Theory (Halo-EFT) framework, in order to study low-energy radiative nucleon capture to a weakly bound (halo) nucleus. Here we focus on the reactions 7Li(n, γ)8Li and 7Be(p, γ)8B, which are subjects of long-standing interest for astrophysics. In the low-energy region we can approximate 8Li (8B) as composed of a 7Li (7Be) core (and also its excitation), and a neutron (proton) with an anomalously extended wave function. The scattering and bound states can be studied in Halo-EFT, in which both core and the nucleon are treated as fundamental degrees of freedom. In our leading order calculation, we use asymptotic normalization coefficients from QMC calculations to fix the parameters in the Lagrangian, which we then apply to study radiative captures. This obviates computing the captures by directly using numerically intensive QMC methods, while still incorporating the nuclear dynamics that these methods provide. In addition, the model-independent EFT framework provides novel insights into the manner in which these two nucleon-capture processes are related to one another. This work is supported by US Department of Energy under grant DE-FG02-93ER-40756.

  1. Microscopic model analysis of the 6He, 6Li+28Si total reaction cross sections at the energy range 5-50 A MeV

    SciTech Connect

    Lukyanov, K. V.; Kukhtina, I. N.; Lukyanov, V. K.; Penionzhkevich, Yu. E.; Sobolev, Yu. G.; Zemlyanaya, E. V.

    2007-05-22

    The existing and some preliminary experimental data on the total cross sections of the 4,6He, 6,7Li+28Si reactions at energies E=5-50 A MeV are demonstrated. The data on 6Li,6He+28Si are analyzed in the framework of the microscopic optical potential with real and imaginary parts obtained with a help of the double-folding procedure and by using the current models of densities of the projectile nuclei. Besides, the microscopic double-folding Coulomb potential is calculated and its effect on cross sections is compared with that when one applies the traditional Coulomb potential of the uniform charge distribution. The semi-microscopic potentials are constructed from both the renormalized microscopic potentials and their derivatives to take into account collective motion effect and to improve an agreement with experimental data.

  2. Production cross section of At radionuclides from 7Li+natPb and 9Be+natTl reactions

    NASA Astrophysics Data System (ADS)

    Maiti, Moumita; Lahiri, Susanta

    2011-12-01

    Earlier we reported theoretical studies on the probable production of astatine radionuclides from 6,7Li- and 9Be-induced reactions on natural lead and thallium targets, respectively. The production of astatine radionuclides were investigated experimentally with two heavy-ion-induced reactions: 9Be + natTl and 7Li + natPb. Formation cross sections of the evaporation residues, 207,208,209,210At, produced in the (HI,xn) channel, were measured by the stacked-foil technique followed by off-line γ spectrometry at low incident energies (<50 MeV). Measured excitation functions were interpreted in terms of a compound nuclear reaction mechanism using Weisskopf-Ewing and Hauser-Feshbach models. Measured cross-section values are lower than the respective theoretical predictions.

  3. Measurements of angular distributions for7Li elastically scattered from58Ni at energies around the Coulomb barrier

    NASA Astrophysics Data System (ADS)

    Amador-Valenzuela, P.; Aguilera, E. F.; Martinez-Quiroz, E.; Lizcano, D.; Morales-Rivera, J. C.

    2017-07-01

    Recently, experimental measurements of elastic scattering angular distributions for the system7Li+58Ni at ten different energies around the Coulomb barrier were made by the Heavy-Ion Group. The measurements were made at the Tandem Van de Graaff Particle Accelerator Laboratory in the National Institute for Nuclear Research (ININ) in Mexico. In this work, preliminary elastic scattering angular distributions for five energies (E lab , = 12.0, 12.5, 13.0, 13.5 and 14.22 MeV) are presented. The preliminary experimental data were analyzed using the São Paulo Optical Model Potential (SPP) which is based on a double-folding potential, reproducing very well these data. A comparison is made with old data reported back in 1973 and in 2012. Further analysis is in progress in order to fully understand this particular system, specially because7Li is known to be a weakly bound nucleus.

  4. Ultracold thermalization of {sup 7}Li and {sup 87}Rb

    SciTech Connect

    Marzok, C.; Deh, B.; Courteille, Ph. W.; Zimmermann, C.

    2007-11-15

    We report on measurements of cross-species thermalization inside a magnetically trapped spin-polarized mixture of {sup 87}Rb and {sup 7}Li atoms with both atoms in their respective low-field-seeking magnetic substates |F=2,m{sub F}=2>. Measurement of the thermalization velocity in the ultracold regime below 10 {mu}K allows for the derivation of the absolute value of the pure triplet s-wave scattering length governing the interaction. We find |a{sub 7,87}|=(59{+-}19)a{sub B}. We propose to study both species in the condensed regime to derive the sign of a{sub 7,87}. In this context, we present numerical solutions to the coupled Gross-Pitaevskii equation based on the hypothesis of a positive sign. According to the simulations, phase separation of the Li and Rb |2,2> clouds occurs along with a mean-field stabilization allowing for larger atom numbers of condensed {sup 7}Li atoms before collapse sets in. Observation of this mean-field stabilization would directly fix the sign of a{sub 7,87}. We discuss our results in the light of this proposal.

  5. Experimental study of π- double charge exchange with 7Li

    NASA Astrophysics Data System (ADS)

    Evseev, V. S.; Kurbatov, V. S.; Sidorov, V. M.; Belyaev, V. B.; Wrzecionko, J.; Daum, M.; Frosch, R.; McCulloch, J.; Steiner, E.

    1981-02-01

    We have observed 150 double charge exchange events, π - + 7Li → π + + anything, at an incident π- lab kinetic energy of 102 MeV. The π+ were recorded in an emulsion stack at 30° to the incident π- beam. No significant peak due to the hypothetical reaction π - + 7Li → π + + 7H(g.s.) was observed in the part of the π+ energy spectrum corresponding to a 7H binding energy between -5 MeV and +25 MeV. Our new upper limit for the corresponding differential cross section is 1.0 × 10 -31{cm 2}/{sr} (90% C.L.). The π+ spectrum was recorded down to low energies (20 MeV < Eπ+ < 100 MeV); its shape implies a strong final-state interaction among the π+, the proton and the six neutrons. The differential double charge exchange cross section integrated over all π+ energies was determined as ( {dσ}/{dΩ}) tot = (4.2 ± 1.7) × 10 -30{cm 2}/{sr}.

  6. Metastable charged sparticles and the cosmological {sup 7}Li problem

    SciTech Connect

    Cyburt, Richard H.; Ellis, John; Luo, Feng; Fields, Brian D.; Olive, Keith A.; Spanos, Vassilis C. E-mail: John.Ellis@cern.ch E-mail: feng.luo@kcl.ac.uk E-mail: spanos@inp.demokritos.gr

    2012-12-01

    We consider the effects of metastable charged sparticles on Big-Bang Nucleosynthesis (BBN), including bound-state reaction rates and chemical effects. We make a new analysis of the bound states of negatively-charged massive particles with the light nuclei most prominent in BBN, and present a new code to track their abundances, paying particular attention to that of {sup 7}Li. Assuming, as an example, that the gravitino is the lightest supersymmetric particle (LSP), and that the lighter stau slepton, τ-tilde {sub 1}, is the metastable next-to-lightest sparticle within the constrained minimal supersymmetric extension of the Standard Model (CMSSM), we analyze the possible effects on the standard BBN abundances of τ-tilde {sub 1} bound states and decays for representative values of the gravitino mass. Taking into account the constraint on the CMSSM parameter space imposed by the discovery of the Higgs boson at the LHC, we delineate regions in which the fit to the measured light-element abundances is as good as in standard BBN. We also identify regions of the CMSSM parameter space in which the bound state properties, chemistry and decays of metastable charged sparticles can solve the cosmological {sup 7}Li problem.

  7. 7Li NMR study of normal human erythrocytes

    NASA Astrophysics Data System (ADS)

    Pettegrew, J. W.; Post, J. F. M.; Panchalingam, K.; Withers, G.; Woessner, D. E.

    The biological action of lithium is of great interest because of the therapeutic efficacy of the cation in manic-depressive illness. To investigate possible molecular interactions of lithium, 7Li NMR studies were conducted on normal human erythrocytes which had been incubated with lithium chloride. The uptake of lithium ions was followed by 7Li NMR, using a dysprosium, tripolyphosphate shift reagent. Lithium uptake followed single-exponential kinetics with a time constant of 14.7 h. The intracellular lithium relaxation times were T 1 ⋍ 5 s and T 2 ⋍ 0.15 s, which implies a lengthening of the lithium correlation time. It was found that lithium does not interact significantly with hemoglobin, the erythrocyte membrane, or artificial phospholipid membranes. Based on measurements of lithium T1 and T2 in concentrated agar gels, the large difference between T1 and T2 for intracellular lithium ions may be due to diffusion of the hydrated lithium ion through heterogeneous electrostatic field gradients created by the erythrocyte membrane-associated cytoskeletal network. Lithium binding to the membrane-associated cytoskeleton, however, cannot be ruled out. Because of the large differences between T1 and T2 of intracellular lithium ions, 1Li NMR may be a sensitive and promising noninvasive method to probe the intracellular environment.

  8. A Study of Five-Nucleon Transfer Mechanisms in the (p, 6Li) Reactions

    NASA Astrophysics Data System (ADS)

    Honda, T.; Kudo, Y.; Horie, H.

    1980-03-01

    The experimental angular distributions for the 5He-transfer reactions 16O(p, 6Li)11C(ground) and 11B(p, 6Li)6Li(ground) at Ep=51.9MeV and analysed in the framework of exact finite-range DWBA formalism with all one-step direct processes. The spectroscopic factors for 16Oto5He+11C, 6Lito p+5He and 11Bto5He+6Li are calculated by making use of cluster coupling shell model wave functions. Good agreements between theoretical calculations and experiments are obtained for both reactions.

  9. A new measurement of the 6Li(n,α)t cross section at MeV energies using a 252Cf fission chamber and 6Li scintillators

    DOE PAGES

    Kirsch, Leo Edward; Devlin, Matthew James; Mosby, Shea Morgan; ...

    2017-09-01

    We present a new measurement of the 6Li(n,α)t cross section from 245 keV to 10 MeV using a 252Cf fission chamber with 6LiI(Eu) and Cs2LiYCl6:Ce (CLYC) scintillators which act as both target and detector. Neutron energies are determined from the time of flight (TOF) method using the signals from spontaneous fission and reaction product recoil. Simulations of neutron downscatter in the crystals and fission chamber bring 6Li(n,α)t cross section values measured with the 6LiI(Eu) into agreement with previous experiments and evaluations, except for two resonances at 4.2 and 6.5 MeV introduced by ENDF/B-VII.1. Suspected neutron transport modeling issues cause themore » cross section values obtained with CLYC to be discrepant above 2 MeV.« less

  10. TLD efficiency of 7LiF for doses deposited by high-LET particles

    NASA Technical Reports Server (NTRS)

    Benton, E. R.; Frank, A. L.; Benton, E. V.

    2000-01-01

    The efficiency of 7 LiF TLDs (TLD-700) in registering dose from high-LET (> or = 10 keV/micrometers) charged particles (relative to 137Cs gamma rays) has been measured for a number of accelerated heavy ions at various particle accelerator facilities. These measured efficiency values have been compared with similar results obtained from the open literature and a dose efficiency function has been fitted to the combined data set. While it was found that the dose efficiency is not only a function of LET, but also of the charge of the incident particle, the fitted function can be used to correct the undermeasured value of dose from exposures made in mixed radiation fields where LET information is available. This LET-dependent dose efficiency function is used in our laboratory in determining total absorbed dose and dose equivalent from combined TLD and CR-39 plastic nuclear track detector measurements.

  11. TLD efficiency of 7LiF for doses deposited by high-LET particles

    NASA Technical Reports Server (NTRS)

    Benton, E. R.; Frank, A. L.; Benton, E. V.

    2000-01-01

    The efficiency of 7 LiF TLDs (TLD-700) in registering dose from high-LET (> or = 10 keV/micrometers) charged particles (relative to 137Cs gamma rays) has been measured for a number of accelerated heavy ions at various particle accelerator facilities. These measured efficiency values have been compared with similar results obtained from the open literature and a dose efficiency function has been fitted to the combined data set. While it was found that the dose efficiency is not only a function of LET, but also of the charge of the incident particle, the fitted function can be used to correct the undermeasured value of dose from exposures made in mixed radiation fields where LET information is available. This LET-dependent dose efficiency function is used in our laboratory in determining total absorbed dose and dose equivalent from combined TLD and CR-39 plastic nuclear track detector measurements.

  12. Study of elastic scattering of mirror nuclei 7Be + 7Li

    NASA Astrophysics Data System (ADS)

    Barua, S.; Das, J. J.; Jhingan, A.; Varughese, T.; Madhavan, N.; Sugathan, P.; Verma, S.; Kalita, K.; Bhattacharjee, B.; Datta, S. K.; Boruah, K.

    2004-12-01

    The angular distribution of 7Be + 7Li elastic scattering has been measured using 7Be from the Radioactive beam at Nuclear Science Centre, New Delhi at E cm = 9.87 MeV. A compact and highly efficient detector system in kinematic coincidence mode and an in-vacuum target transfer system have been developed to minimise contributions from unwanted channels. The angular ranges covered were θcm = 42°- 66°and θcm = 114°- 138°. The experimental angular distribution shows higher cross sections than the theoretical predictions at the backward angles. The experimental data could be fitted with an isospin dependent complex potential that is analogous to the Lane potential.

  13. Most frequent value statistics and distribution of 7Li abundance observations

    NASA Astrophysics Data System (ADS)

    Zhang, J.

    2017-07-01

    The problem of primordial lithium is one of the key issues in many astrophysical fields, especially nuclear astrophysics and cosmology. We apply a novel modern statistical method - the most frequent value (MFV) procedure - to study the distribution modelling for 7Li abundance observations, constructing a robust and effective astrostatistical algorithm. Considering prior non-Gaussian error distributions of measurements of astrophysical quantities, the robust MFV method is essential as a standard statistical algorithm, according to the minimization for the information loss principle. Associated with global optimization, the MFV procedure has already been shown to be a more powerful tool than some classic statistical algorithms originating from the least-squares or maximum likelihood principle for dealing with the unknown distribution problems of observed astrophysical quantities. Applying the MFV algorithm, we obtain the MFV M = 2.205 and the dihesion ɛ = 0.067 of A(Li) measurements, which demonstrate certain advantages to solving problems with a non-Gaussian error distribution.

  14. Toward Simultaneous Quantum Degeneracy of ^133Cs and ^6Li Atoms

    NASA Astrophysics Data System (ADS)

    Sharma, Arjun; Degenkolb, Skyler; Gemelke, Nathan; Brickman Soderberg, Kathy-Anne; Chin, Cheng

    2010-03-01

    A quantum degenerate mixture of ^133Cs and ^6Li atoms provides interesting prospects to investigate few- and many-body physics and to realize quantum information processing. Simultaneous evaporative cooling of bosonic ^133Cs and fermionic ^6Li is challenging. In an optical dipole trap formed with a 1064nm laser, ^133Cs (resonant transition at 852nm) experiences a deeper potential than ^6Li (at 671nm). Since laser cooling allows a much lower initial temperature for ^133Cs (10μK) than for ^6Li (150μK), a wide, shallow trap optimizes ^133Cs loading, but ^6Li requires a deep trap. Efficient cooling of ^6Li involves Feshbach resonance tuning near 800G, but ^133Cs collision properties are untested at high fields. Furthermore, sympathetic cooling of ^6Li by ^133Cs can suffer from the large mass ratio causing imperfect overlap of clouds and slow collisional rethermalization. We report our work toward collision studies of ^133Cs -^6Li and ^133Cs-^133Cs in fields up to 1000G and its implications for optimal evaporation, as well as the implementation of quantum gate operations.

  15. {sup 16}O resonances near 4α threshold through {sup 12}C({sup 6}Li,d) reaction

    SciTech Connect

    Rodrigues, M. R. D.; Borello-Lewin, T.; Miyake, H.; Horodynski-Matsushigue, L. B.; Duarte, J. L. M.; Rodrigues, C. L.; Faria, P. Neto de; Cunsolo, A.; Cappuzzello, F.; Foti, A.; Agodi, C.; Cavallaro, M.; Napoli, M. di; Ukita, G. M.

    2014-11-11

    Several narrow alpha resonant {sup 16}O states were detected through the {sup 12}C({sup 6}Li,d) reaction, in the range of 13.5 to 17.5 MeV of excitation energy. The reaction was measured at a bombarding energy of 25.5 MeV employing the São Paulo Pelletron-Enge-Spectrograph facility and the nuclear emulsion technique. Experimental angular distributions associated with natural parity quasi-bound states around the 4α threshold are presented and compared to DWBA predictions. The upper limit for the resonance widths obtained is near the energy resolution (15 keV)

  16. Importance of the continuum-continuum couplings in the 6Li elastic breakup on different target masses

    NASA Astrophysics Data System (ADS)

    Mukeru, B.; Lekala, M. L.

    2017-09-01

    A theoretical study of 6Li breakup on target masses ranging from A = 58 to 208 is performed. It is obtained that when continuum-continuum couplings are included in the potential coupling matrix, they substantially reduce the total and nuclear breakup cross sections, while the Coulomb breakup cross sections for the medium and heavy target masses are increased. When these couplings are excluded, we show that the total and nuclear breakup cross sections depend linearly on AT1/3, namely they decrease linearly as the mass of the target increases. In the same case, the Coulomb breakup cross section depends linearly with the charge of the target ZT (decreases as ZT increases). We found that this linearity is destroyed when these couplings are included. However, in this case, it is the Coulomb-nuclear interference that also depends linearly with the target charge (increase with ZT).

  17. Acute CNS syndrome from /sup 10/B(n,. cap alpha. )/sup 7/Li irradiation of mouse brain

    SciTech Connect

    Slatkin, D.N.; Stoner, R.D.; Rosander, K.M.; Kalef-Ezra, J.K.; Laissue, J.A.

    1986-01-01

    The purpose of this study is to compare absorbed doses of /sup 10/B-neutron capture radiation and x radiation in the brains of head-exposed, body-shielded mice, at LD/sub 50/ for acute (<4 days post exposure) mortality from the central nervous system (CNS) radiation syndrome. This comparison leads to an estimate of the in vivo relative biological effectiveness (RBE) of heavy particle radiation (helium and lithium ions) from the /sup 10/B(n,..cap alpha..)/sup 7/Li nuclear reaction.

  18. Non-Gaussian error distribution of 7Li abundance measurements

    NASA Astrophysics Data System (ADS)

    Crandall, Sara; Houston, Stephen; Ratra, Bharat

    2015-07-01

    We construct the error distribution of 7Li abundance measurements for 66 observations (with error bars) used by Spite et al. (2012) that give A(Li) = 2.21 ± 0.065 (median and 1σ symmetrized error). This error distribution is somewhat non-Gaussian, with larger probability in the tails than is predicted by a Gaussian distribution. The 95.4% confidence limits are 3.0σ in terms of the quoted errors. We fit the data to four commonly used distributions: Gaussian, Cauchy, Student’s t and double exponential with the center of the distribution found with both weighted mean and median statistics. It is reasonably well described by a widened n = 8 Student’s t distribution. Assuming Gaussianity, the observed A(Li) is 6.5σ away from that expected from standard Big Bang Nucleosynthesis (BBN) given the Planck observations. Accounting for the non-Gaussianity of the observed A(Li) error distribution reduces the discrepancy to 4.9σ, which is still significant.

  19. Studies of the Efimov Effect in 7 Li

    NASA Astrophysics Data System (ADS)

    Luo, D.; Nguyen, J. H. V.; Hulet, R. G.

    2016-05-01

    Ultracold atomic gases provide an ideal environment to study few body physics in the universal regime. Passive techniques, such as monitoring loss of the atomic sample while varying the hold time allows us to explore properties such as the scaling behavior of Efimov trimers. In our experiment, we explore how the Efimov states are affected by non-zero temperature. We measure the three-body loss rate for a 7 Li atom gas at different scattering lengths and extract the location and width of an Efimov recombination minimum for various temperatures. Alternatively, we may perform more active experiments such as creating dimers using RF-field modulation as a probe of molecular binding energies. We use RF-association to form Feshbach dimers and Efimov trimers, and find a strong enhancement of the dimer formation rate at the atom-dimer resonance, which could be explained by an avalanche mechanism. In the past the enhancement in the three-body recombination rate at the same location had also been observed, and attributed to the avalanche. We explore the link between these findings with a side-by-side comparison of the dimer-formation rate and the three-body loss rate. Work supported by the NSF, an ARO MURI Grant, and the Welch Foundation.

  20. Use of 7Li(p,n) reaction as a neutron source in a PGNAA setup.

    PubMed

    Naqvi, A A; Nagadi, M M

    2005-03-01

    The performance of a 7Li(p,n) reaction-based Prompt Gamma Ray Neutron Activation Analysis (PGNAA) setup has been determined for analysis of Portland cement samples using Monte Carlo study. The calculations were carried out for a 7Li(p,n) reaction-based PGNAA setup with an external moderator similar to the one used in a previous 2.8 MeV neutrons-based PGNAA setup. The optimum values of geometry parameters of the 7Li(p,n) reaction-based setup are different from those of the 2.8 MeV neutrons-based setup resulting in better performance of the 7Li(p,n) reaction-based setup. The prompt gamma-ray yield from the 7Li(p,n) reaction-based setup is 60-70% higher than that from the 2.8 MeV neutrons-based setup. Although the performances of the 7Li(p,n) reaction-based setup is comparable with that of a previously studied 3H(p,n) reaction-based setup, yet performance of the 7Li(p,n) reaction-based setup is superior to that of the 3H(p,n) reaction-based setup because it has less radiation hazard due to utilization of non-radioactive neutron producing target. This study has provided a theoretical base for experimental test of a 7Li(p,n) reaction-based PGNAA setup.

  1. Prospects of lithium enrichment on 7Li isotope by method of controlled ions electro-migration

    NASA Astrophysics Data System (ADS)

    Martoyan, G. A.; Kalugin, M. M.; Gabrielyan, A. V.; Martoyan, A. G.

    2016-01-01

    This paper deals with a new electro-membrane method of enrichment of 7Li isotope. The data are presented on the importance and application fields regarding the use of 7Li isotopes. Existing methods and criteria of separation of lithium isotopes are discussed. The principle of new technology, regimes of enrichment experiments, and analysis details of obtained products are briefly described.

  2. Influence of the {alpha}-d motion in {sup 6}Li on Trojan horse applications

    SciTech Connect

    Pizzone, R.G.; Spitaleri, C.; Cherubini, S.; La Cognata, M.; Lamia, L.; Musumarra, A.; Romano, S.; Tumino, A.; Tudisco, S.; Miljanic, D.; Typel, S.

    2005-05-01

    The {alpha}-d cluster structure of {sup 6}Li has been extensively investigated in the past few decades. In particular the width of the {alpha} momentum distribution in {sup 6}Li has been studied as a function of the transferred momentum. These investigations are now reviewed and updated after recent experiments. Trojan horse method applications are also discussed because the momentum distribution of the spectator particle inside the Trojan horse nucleus is a necessary input for this method. The impact of the width (FWHM) variation in the extraction of the astrophysical S(E) factor is discussed for the {sup 6}Li(d,{alpha}){sup 4}He reaction.

  3. Basic technology for 6Li enrichment using an ionic-liquid impregnated organic membrane

    NASA Astrophysics Data System (ADS)

    Hoshino, Tsuyoshi; Terai, Takayuki

    2011-10-01

    The tritium needed as a fuel for fusion reactors is produced by the neutron capture reaction of lithium-6 ( 6Li) in tritium breeding materials. However, natural Li contains only about 7.6 at.% 6Li. In this paper, a new lithium isotope separation technique using an ionic-liquid impregnated organic membrane is proposed. In order to separate and concentrate lithium isotopes, only lithium ions are able to move through the membrane by electrodialysis between the cathode and the anode in lithium solutions. Preliminary experiments of lithium isotope separation were conducted using this phenomenon. Organic membranes impregnated with TMPA-TFSI and PP13-TFSI as ionic liquids were prepared, and the relationship between the 6Li separation coefficient and the applied electrodialytic conditions was evaluated using them. The results showed that the 6Li isotope separation coefficient in this method (about 1.1-1.4) was larger than that in the mercury amalgam method (about 1.06).

  4. {sup 6}LiF oleic acid capped nanoparticles entrapment in siloxanes for thermal neutron detection

    SciTech Connect

    Carturan, S. Maggioni, G.; Marchi, T.; Gramegna, F.; Cinausero, M.; Quaranta, A.; Palma, M. Dalla

    2016-07-07

    The good light output of siloxane based scintillators as displayed under γ-rays and α particles has been exploited here to obtain clear and reliable response toward thermal neutrons. Sensitization towards thermal neutrons has been pursued by adding {sup 6}LiF, in form of nanoparticles. Aiming at the enhancement of compatibility between the inorganic nanoparticles and the low polarity, siloxane based surrounding medium, oleic acid-capped {sup 6}LiF nanoparticles have been synthesized by thermal decomposition of Li trifluoroacetate. Thin pellets siloxane scintillator maintained their optical transmittance up to weight load of 2% of {sup 6}Li. Thin samples with increasing {sup 6}Li concentration and thicker ones with fixed {sup 6}Li amount have been prepared and tested with several sources (α, γ-rays, moderated neutrons). Light output as high as 80% of EJ212 under α irradiation was measured with thin samples, and negligible changes have been observed as a result of {sup 6}LiF addition. In case of thick samples, severe light loss has been observed, as induced by opacity. Nevertheless, thermal neutrons detection has been assessed and the data have been compared with GS20, based on Li glass, taken as a reference material.

  5. A critical evaluation of heteronuclear TOCSY (HEHAHA) experiments for 1H,6Li spin pairs.

    PubMed

    Bergander, Klaus; Hüls, Dietmar; Glaser, Steffen J; Günther, Harald; Luy, Burkhard

    2014-12-01

    Heteronuclear TOCSY (HEHAHA) experiments for (1) H,(6) Li spin pairs in organolithium compounds with adjacent strongly coupled (1) H,(1) H spin systems showed unexpected cross peak behaviour: for n-butyllithium (1) H,(6) Li cross peaks were completely missing, whereas for the dimer of (Z)-2-lithio-1-(o-lithiophenyl)ethane, a cross peak for remote protons was observed even at very short mixing times. It was assumed that strong magnetization transfer within the proton spin systems was responsible for these results, which prevented unambiguous chemical shift assignments. Selective experiments with the (6) Li,(1) H-HET-PLUSH-TACSY sequence then showed the expected (6) Li,(1) H cross peaks for the transfer via the directly coupled (1) H and (6) Li nuclei. For n-butyllithium transfer to H(Cα) via an unresolved heteronuclear coupling constant below 0.1 Hz is unambiguously observed. Cross peaks in the 2D (6) Li,(1) H-HET-PLUSH-TACSY spectra for the dimer of (Z)-2-lithio-1-(o-lithiophenyl)ethane are readily explained by the measured coupling network and the corresponding active mixing conditions.

  6. 6LiF oleic acid capped nanoparticles entrapment in siloxanes for thermal neutron detection

    NASA Astrophysics Data System (ADS)

    Carturan, S.; Maggioni, G.; Marchi, T.; Gramegna, F.; Cinausero, M.; Quaranta, A.; Palma, M. Dalla

    2016-07-01

    The good light output of siloxane based scintillators as displayed under γ-rays and α particles has been exploited here to obtain clear and reliable response toward thermal neutrons. Sensitization towards thermal neutrons has been pursued by adding 6LiF, in form of nanoparticles. Aiming at the enhancement of compatibility between the inorganic nanoparticles and the low polarity, siloxane based surrounding medium, oleic acid-capped 6LiF nanoparticles have been synthesized by thermal decomposition of Li trifluoroacetate. Thin pellets siloxane scintillator maintained their optical transmittance up to weight load of 2% of 6Li. Thin samples with increasing 6Li concentration and thicker ones with fixed 6Li amount have been prepared and tested with several sources (α, γ-rays, moderated neutrons). Light output as high as 80% of EJ212 under α irradiation was measured with thin samples, and negligible changes have been observed as a result of 6LiF addition. In case of thick samples, severe light loss has been observed, as induced by opacity. Nevertheless, thermal neutrons detection has been assessed and the data have been compared with GS20, based on Li glass, taken as a reference material.

  7. Production of beams from solid materials at Center for Nuclear Study electron cyclotron resonance ion source.

    PubMed

    Ohshiro, Y; Yamaka, S; Watanabe, S; Kobayashi, K; Kotaka, Y; Nishimura, M; Kase, M; Muto, H; Yamaguchi, H; Shimoura, S

    2014-02-01

    Two methods for the feed of vapor from solid materials in the Center for Nuclear Study ECR ion source are described. A rod placed near the wall of the plasma chamber, operating up to a melting point of 2600 °C, has been used for CaO, SiO2, and FeO. An oven with a number of openings, operating up to 800 °C, has been used for P2O5, Li, and S. Typical ion beam intensities of (7)Li(2+), (6)Li(3+), (40)Ca(12+), and (56)Fe(15+) are achieved 280, 75, 28, and 7 eμA, respectively. High intensity heavy ion beams are stably supplied into the azimuthally varying field cyclotron.

  8. Determining the 7Li(n,γ) cross section via Coulomb dissociation of 8Li

    NASA Astrophysics Data System (ADS)

    Izsák, R.; Horváth, Á.; Kiss, Á.; Seres, Z.; Galonsky, A.; Bertulani, C. A.; Fülöp, Zs.; Baumann, T.; Bazin, D.; Ieki, K.; Bordeanu, C.; Carlin, N.; Csanád, M.; Deák, F.; DeYoung, P.; Frank, N.; Fukuchi, T.; Gade, A.; Galaviz, D.; Hoffman, C. R.; Peters, W. A.; Schelin, H.; Thoennessen, M.; Veres, G. I.

    2013-12-01

    The applicability of Coulomb dissociation reactions to determine the cross section for the inverse neutron capture reaction was explored using the reaction 8Li(γ,n)7Li. A 69.5 MeV/nucleon 8Li beam was incident on a Pb target, and the outgoing neutron and 7Li nucleus were measured in coincidence. The deduced (n,γ) excitation function is consistent with data for the direct capture reaction 7Li(n,γ)8Li and with low-energy effective field theory calculations.

  9. Inelastic neutron scattering cross-section measurements on 7Li and 63,65Cu

    NASA Astrophysics Data System (ADS)

    Nyman, Markus; Belloni, Francesca; Ichinkhorloo, Dagvadorj; Pirovano, Elisa; Plompen, Arjan; Rouki, Chariklia

    2017-09-01

    The γ-ray production cross section for the 477.6-keV transition in 7Li following inelastic neutron scattering has been measured from the reaction threshold up to 18 MeV. This cross section is interesting as a possible standard for other inelastic scattering measurements. The experiment was conducted at the Geel Electron LINear Accelerator (GELINA) pulsed white neutron source with the Gamma Array for Inelastic Neutron Scattering (GAINS) spectrometer. Previous measurements of this cross section are reviewed and compared with our results. Recently, this cross section has also been calculated using the continuum discretized coupled-channels (CDCC) method. Experiments for studying neutrinoless double-β decay (2β0ν) or other very rare processes require greatly reducing the background radiation level (both intrinsic and external). Copper is a common shielding and structural material, used extensively in experiments such as COBRA, CUORE, EXO, GERDA, and MAJORANA. Understanding the background contribution arising from neutron interactions in Cu is important when searching for very weak experimental signals. Neutron inelastic scattering on natCu was investigated with GAINS. The results are compared with previous experimental data and evaluated nuclear data libraries.

  10. Nucleon and triton production from nucleon-induced reactions on 7Li

    NASA Astrophysics Data System (ADS)

    Watanabe, Yukinobu; Guo, Hairui; Nagaoka, Kohei; Matsumoto, Takuma; Ogata, Kazuyuki; Yahiro, Masanobu

    2016-06-01

    Nucleon (N) and triton production from nucleon-induced reactions on 7Li at an incident energy of 14 MeV are analyzed by using three-body continuum discretized coupled channels method (CDCC), final state interaction (FSI) model, and sequential decay (SD) model. The CDCC is used to describe nucleon and triton production via breakup continuum channels, 7Li(N,N')7Li*→ t + α. Triton production from p(n) + 7Li → t + 5Li(5He) channel and nucleon production from sequential decay of the ground-state 5Li(5He) are calculated by the FSI model and the SD model, respectively. The calculated double differential cross sections for both nucleon and triton production are in good agreement with experimental ones except at relatively low nucleon emission energies.

  11. The ^12C(^6Li,d)^16O reaction at 34 MeV

    NASA Astrophysics Data System (ADS)

    Mendez, A. J.; Brune, C. R.; Karwowski, H. J.; Ludwig, E. J.; Veal, K. D.; Bartosz, E. E.; Cathers, P. D.; Drummer, T. L.; Kemper, K. W.; Koslowska, B.

    1996-05-01

    Present models of the ^6Li nucleus are in disagreement(D. R. Lehman, Colloque de Physique suppl. n22, 52), C6-47 (1990).^,(A. M. Eiro et al.), Few Body Systems suppl. 99 (1995). as to the sign of the D- to S-state ratio, η. Transfer reactions induced by polarized ^6Li have been predicted^3 to be sensitive to η, and recent measurements(A. J. Mendez et al.), Phys. Rev. C 51, 651 (1995). have shown a sensitivity to the presence of the D-state in ^6Li. We will present cross-section, A_y, and A_zz angular-distribution measurements for the ^12C(^6Li,d)^16O reaction at 34 MeV over the laboratory angular range 6.5^circ - 60^circ. We find Ay to be large, negative and highly oscillatory for the 0^+ ground state and predominantly negative, but smaller and less oscillatory, for both the 3^- state at 6.13 MeV and the 2^+, 1^- doublet at 7 MeV. The A_zz distributions for the first two states are large and oscillatory about zero, while that of the doublet is predominantly negative. We will present a DWBA analysis of the data and discuss the consequences for η(^6Li).

  12. Alpha Resonances in {sup 13}C Excited by the {sup 9}Be ({sup 6}Li,d) Reaction

    SciTech Connect

    Rodrigues, M. R. D.; Borello-Lewin, T.; Horodynski-Matsushigue, L. B.; Duarte, J. L. M.; Rodrigues, C. L.; Souza, M. A.; Miyake, H.; Cunsolo, A.; Cappuzzello, F.; Ukita, G. M.

    2010-05-21

    The {sup 9}Be({sup 6}Li,d){sup 13}C reaction was used to investigate alpha resonant states in {sup 13}C up to 13 MeV of excitation. The reaction was measured at a bombarding energy of 25.5 MeV employing the Sao Paulo Pelletron-Enge-Spectrograph facility and the nuclear emulsion detection technique. The resolution of 50 keV allowed for the separation of the resonant contributions to the known 7/2{sup -} at 10.753 MeV and (5/2{sup -}) at 10.818 MeV {sup 13}C states. The alpha resonance seen at the (3alpha+n) threshold was not previously reported. The experimental angular distributions are presented in comparison with DWBA predictions.

  13. 6Li-loaded directionally sensitive anti-neutrino detector for possible geo-neutrinographic imaging applications

    PubMed Central

    Tanaka, H. K. M.; Watanabe, H.

    2014-01-01

    Despite the latent and unique benefits of imaging uranium and thorium's distribution in the earth's interior, previously proposed experimental techniques used to identify the incoming geo-neutrino's direction are not applicable to practical imaging due to the high miss-identification in a neutrino's track reconstruction. After performing experimental studies and Monte-Carlo simulations, we confirmed that a significant improvement is possible in neutrino tracking identification with a 6Li-loaded neutrino detector. For possible imaging applications, we also explore the feasibility of producing geo-neutrinographic images of gigantic magmatic reservoirs and deep structure in the mantle. We anticipate and plan to apply these newly designed detectors to radiographic imaging of the Earth's interior, monitoring of nuclear reactors, and tracking astrophysical sources of neutrinos. PMID:24759616

  14. Elastic, inelastic, and 1-nucleon transfer channels in the 7Li+120Sn system

    NASA Astrophysics Data System (ADS)

    Kundu, A.; Santra, S.; Pal, A.; Chattopadhyay, D.; Tripathi, R.; Roy, B. J.; Nag, T. N.; Nayak, B. K.; Saxena, A.; Kailas, S.

    2017-03-01

    Background: Simultaneous description of major outgoing channels for a nuclear reaction by coupled-channels calculations using the same set of potential and coupling parameters is one of the difficult tasks to accomplish in nuclear reaction studies. Purpose: To measure the elastic, inelastic, and transfer cross sections for as many channels as possible in 7Li+120Sn system at different beam energies and simultaneously describe them by a single set of model calculations using fresco. Methods: Projectile-like fragments were detected using six sets of Si-detector telescopes to measure the cross sections for elastic, inelastic, and 1-nucleon transfer channels at two beam energies of 28 and 30 MeV. Optical model analysis of elastic data and coupled-reaction-channels (CRC) calculations that include around 30 reaction channels coupled directly to the entrance channel, with respective structural parameters, were performed to understand the measured cross sections. Results: Structure information available in the literature for some of the identified states did not reproduce the present data. Cross sections obtained from CRC calculations using a modified but single set of potential and coupling parameters were able to describe simultaneously the measured data for all the channels at both the measured energies as well as the existing data for elastic and inelastic cross sections at 44 MeV. Conclusions: Non-reproduction of some of the cross sections using the structure information available in the literature which are extracted from reactions involving different projectiles indicates that such measurements are probe dependent. New structural parameters were assigned for such states as well as for several new transfer states whose spectroscopic factors were not known.

  15. Alpha spectroscopic factors from (12)C((6)->Li,d): A thirty year mystery

    NASA Astrophysics Data System (ADS)

    Drummer, Timothy Lee

    1998-10-01

    Polarized 6Li beams have been used to study the α-transfer reaction 12C(6Li,d)16O at 6Li bombarding energies of 34 and 50 MeV. The experiments were carried out at the FSU Tandem Van de Graaf/Superconducting Linear Accelerator Laboratory. A complete set of analyzing powers (iT11, T20, T21, and T22) for transfers to the ground, 3-(6.13 MeV), 2+ (6.92 MeV), and 4+ (10.35 MeV) states of 16O have been measured using the Optically Pumped Polarized Lithium Ion Source (OPPLIS). A new PC based computer data acquisition system was developed, tested, and employed to conduct these measurements. The measured analyzing powers to states in 16O are large. A Finite-Range Distorted Wave Born Approximation (FRDWBA) analysis using central, spin orbit, and tensor scattering potentials has been conducted to understand the measured 12C(6Li,d) data. The ground state 0+ /to 0+ transfer analyzing powers are a sensitive tool for studying the reaction mechanism. The scattering potential parameters were selected such that the 12C(6Li,d) calculations reproduced both the transfer data, as well as the available 6Li + 12C and d + 16O elastic scattering data. While 6Li is predominantly composed of α + d clusters in a relative S-state, the FRDWBA calculations also included the effects of the D-state contribution in the 6Li wavefunction. The calculations investigated the dependence of the calculated angular distributions on the 12C + α bound state radius. The FRDWBA calculations showed that the 16O(g.s.) analyzing powers are the result of the deuteron spin orbit potential term in the d + 16O exit channel. The 16O excited state analyzing powers were not reproduced by the FRDWBA calculations. Alpha spectroscopic factors and reduced widths were extracted for all the measured states of 16O. Coupled Channels Born Approximation (CCBA) calculations were performed using a double folded real potential for the 6Li + 12C entrance channel interaction. Ten inelastic channels in the 6Li + 12C and d + 16O

  16. Properties of 4He and 6Li with improved chiral EFT interactions

    NASA Astrophysics Data System (ADS)

    Maris, P.; Binder, S.; Calci, A.; Epelbaum, E.; Furnstahl, R. J.; Golak, J.; Hebeler, K.; Kamada, H.; Krebs, H.; Langhammer, J.; Liebig, S.; Meißner, U.-G.; Minossi, D.; Nogga, A.; Potter, H.; Roth, R.; Skibiński, R.; Topolnicki, K.; Vary, J. P.; Witala, H.

    2016-03-01

    We present recent results for 4He and 6Li obtained with improved NN interactions derived from chiral effective field theory up to N4LO. The many-body calculations are performed order-by-order in the chiral expansion. At N3LO and N4LO additional renormalization using the Similarity Renormalization Group is adopted to improve numerical convergence of the many-body calculations. We discuss results for the ground state energies, as well as the magnetic moment and the low-lying spectrum of 6Li.

  17. OMPs for the 6 He + 209 Bi halo system from a 208 Pb(7 Li,6 He)209 Bi reaction analysis

    NASA Astrophysics Data System (ADS)

    Yang, L.; Lin, C. J.; Jia, H. M.; Wang, D. X.; Sun, L. J.; Ma, N. R.; Yang, F.; Wu, Z. D.; Xu, X. X.; Zhang, H. Q.; Liu, Z. H.; Bao, P. F.

    2017-09-01

    Angular distributions of transfer reaction {^{208}} Pb( 7 Li, {6} He) {^{209}} Bi were measured at E_{{lab}} ( {^7} Li)= 21.2 , 24.3, 25.67 and 28.55MeV. By fitting the experimental data with the theoretical frameworks of Distorted Wave Born Approximation (DWBA), the optical model parameters of the halo nuclear system 6 He + 209 Bi were extracted. The breakup threshold anomaly (BTA) was observed clearly in the imaginary potential, and a further decreasing trend in the deep sub-barrier region was observed for the first time in a halo system. Furthermore, the dispersion relation is found of no use to describe the connection between the real and imaginary parts.

  18. Thermal neutron calibration of a tritium extraction facility using the /sup 6/Li(n,t)/sup 4/He//sup 197/Au(n,. gamma. )/sup 198/Au cross section ratio for standardization

    SciTech Connect

    Bretscher, M.M.; Smith, D.L.

    1980-08-01

    Absolute tritium activities in a neutron-activated metallic lithium samples have been measured by liquid scintillation methods to provide data needed for the determination of capture-to-fission ratios in fast breeder reactor spectra and for recent measurements of the /sup 7/Li(n,n't)/sup 4/He cross section. The tritium extraction facility used for all these experiments has now been calibrated by measuring the /sup 6/Li(n,t)/sup 4/He//sup 197/Au/n,..gamma..)/sup 198/Au activity ratio for thermal neutrons and comparing the result with the well-known cross sections. The calculated-to-measured activity ratio was found to be 1.033 +- 0.018. 2 figures, 20 tables.

  19. Fourier transform spectroscopy of the 1 3Sigma + g-a 3Sigma + u transition of the 6Li2 molecule

    NASA Astrophysics Data System (ADS)

    Linton, C.; Murphy, T. L.; Martin, F.; Bacis, R.; Verges, J.

    1989-11-01

    The 1 3Σ+g-a 3Σ+u transition of 6Li2 has been observed via collisionally induced fluorescence, excited by visible lines of an argon-ion laser and detected at high resolution with a Fourier-transform spectrometer in the 8200-10 100 cm-1 region. By combining the results with previously obtained data on 7Li2 [F. Martin, R. Bacis, J. Vergès, C. Linton, G. Bujin, C. H. Cheng, and E. Stad, Spectrochim. Acta Part A 44, 1369 (1988)], an accerate, isotopically consistent description of both states has been obtained for 1≤v'≤7 and 0≤v`≤7. Equilibrium constants, Rydberg-Klein-Rees potential curves, and dissociation energies have been determined and found to be in good agreement with ab initio calculations. From the analysis, the following positions and dissociation energies of the two states were found. For 1 3Σ+g, Te (cm-1) is 16 328.8(1.7) and De (cm-1) is 7091.6(1.2). For a 3Σ+u, Te (cm-1) is 8183.8(1.5) and De (cm-1) is 333(1).

  20. New study of the astrophysical reaction 13C(a,n)16O via the 13C(7Li,t)17O transfer reaction

    NASA Astrophysics Data System (ADS)

    Pellegriti, Maria Grazia; Hammache, F.; Roussel, P.; Audouin, L.; Beaumel, D.; Fortier, S.; Gaudefroy, L.; Kiener, J.; Lefebvre-Schujl, A.; Stanoiu, M.; Tatischeff, V.; Vilmay, M.

    PoS(NIC-IX)161 , , [1] , L. Gaudefroy[2] , J. Kiener[3] , A. Lefebvre-Schuhl[3] , M. Stanoiu[4] , V. The cross section of the 13 C(α,n)16 O reaction is a key ingredient for the comprehension of the s-process (slow neutron captures) in stars. This reaction is considered as the main neutron source for the s-process in low-mass Asymptotic Giant Branch (AGB) stars (1-3 solar mass) [1, 2, 3]. At the α-13 C energies of astrophysical interest (Ecm around 190 keV, corresponding to a tem- perature of 108 K) the contribution of the 17 O α-decay subthreshold resonance at 6.356 MeV to the 13 C(α,n)16 O cross section should be taken into account. The effect of this resonance is controversial after the different analyses of the Kubono et al. measurement [4] of the 6.356 MeV α-spectroscopic factor (Sα ) via the transfer reaction 13 C(6 Li,d)17 O . In order to further investigate the contribution of the 6.356 MeV resonance to the 13 C(α,n)16 O cross section, we performed a new measurement of its Sα factor via a different α-transfer reac- tion, namely the 13 C(7 Li,t)17 O reaction. The experiment was performed at the Orsay Tandem by using a 7 Li beam of 28 and 34 MeV on a 13C target. The angular distribution for the transfer dif- ferential cross section was measured by detecting the tritons at the focal plane of the SPLITPOLE spectrometer. The analysis procedure used in order to extract the yield of the 6.356 MeV level will be described. Preliminary results of the angular distribution will be shown.

  1. Generation 6 Li-Ion Cell Vibration Testing at ABSL Space Products

    NASA Astrophysics Data System (ADS)

    Defer, M.; Borthomieu, Y.; Ligneel, E.; Badet, S.

    2014-08-01

    This paper presents the design of Saft's Generation6 Li-Ion cell, the main challenges in the course of the development, the main BOL characteristics and performances achieved during the development program. Finally, it also describes how this cell fits in Saft's battery range and the benefits of it.

  2. A quantum degenerate Bose-Fermi mixture of 41K and 6Li

    NASA Astrophysics Data System (ADS)

    Wu, Yu-Ping; Yao, Xing-Can; Chen, Hao-Ze; Liu, Xiang-Pei; Wang, Xiao-Qiong; Chen, Yu-Ao; Pan, Jian-Wei

    2017-05-01

    We report a new apparatus for the study of two-species quantum degenerate mixture of 41K and 6Li atoms. We develop and combine several advanced cooling techniques to achieve both a large atom number and high phase space density of the two-species atom clouds. Furthermore, we build a high efficiency two-species magnetic transport system to transfer atom clouds from the 3D magneto-optical-trap chamber to a full glass science chamber of an extreme high vacuum environment and good optical access. We perform a forced radio-frequency evaporative cooling for 41K atoms while the 6Li atoms are sympathetically cooled in an optically plugged magnetic trap. Finally, we achieve the simultaneous quantum degeneracy for the 41K and 6Li atoms. The Bose-Einstein condensate of 41K has 1.4 × 105 atoms with a condensate fraction of about 62%, while the degenerate Fermi gas of 6Li has a total atom number of 5.4 × 105 at 0.25 Fermi temperature.

  3. Nuclear Reactions in Hot Astrophysical Plasmas with T > 1010 K

    NASA Astrophysics Data System (ADS)

    Kafexhiu, Ervin; Aharonian, Felix; Vila, Gabriela S.

    The importance of nuclear reactions in low-density astrophysical plasmas with ion temperatures T ≥1010 K has been recognized for more than thirty years. However, the lack of comprehensive data banks of relevant nuclear reactions and the limited computational power have not previously allowed detailed theoretical studies. Recent developments in these areas make it timely to conduct comprehensive studies on the nuclear properties of very hot plasmas formed around compact relativistic objects such as black holes and neutron stars. Such studies are of great interest in the context of scientific programs of future low-energy cosmic γ-ray spectrometry. In this work, using the publicly available code TALYS, we have built a large nuclear network relevant for temperatures exceeding 1010 K. We have studied the evolution of the chemical composition and accompanying prompt gamma-ray emission of such high-temperature plasmas. We present the results on the abundances of light elements D, T, 3He, 4He, 6Li, 7Li, 9Be, 10B, 11B, and briefly discuss their implications on the astrophysical abundances of these elements.

  4. The interstellar Li-7/Li-6 isotope ratio toward Zeta Ophiuchi and Zeta Persei

    NASA Technical Reports Server (NTRS)

    Meyer, David M.; Hawkins, Isabel; Wright, Edward L.

    1993-01-01

    High S/N, high-resolution observations of the interstellar Li absorption lines toward the stars Zeta Ophiuchi and Zeta Persei are reported. Li I line profiles indicate the presence of both the Li-7 and Li-6 doublets in these two sightlines. Best-fit values for the interstellar Li-7/Li-6 isotope ratio are 6.8 (+1.4/-1.7) towards Zeta Ophiuchi and 5.5 (+ 1.3/-1.1) toward Zeta Persei. Measurement of 6.8 (+1.4/-1.7) for the interstellar Li-7/Li-6 isotope ratio towards Zeta Ophiuchi does not support the lower limit of 25 determined by Ferlet and Dennefeld (1984). The current value of the interstellar Li-7/Li-6 isotope ratio is the result of various lithium production and destruction processes involving stars, cosmic rays, and the big bang.

  5. Lithium Visibility in Rat Brain and Muscle in Vivoby 7Li NMR Imaging

    NASA Astrophysics Data System (ADS)

    Komoroski, Richard A.; Pearce, John M.; Newton, Joseph E. O.

    1998-07-01

    The apparent concentration of lithium (Li)in vivowas determined for several regions in the brain and muscle of rats by7Li NMR imaging at 4.7 T with inclusion of an external standard of known concentration and visibility. The average apparent concentrations were 10.1 mM for muscle, and 4.2-5.3 mM for various brain regions under the dosing conditions used. The results were compared to concentrations determinedin vitroby high-resolution7Li NMR spectroscopy of extracts of brain and muscle tissue from the same rats. The comparison provided estimates of the7Li NMR visibility of the Li cation in each tissue region. Although there was considerable scatter of the calculated visibilities among the five rats studied, the results suggested essentially full visibility (96%) for Li in muscle, and somewhat reduced visibility (74-93%) in the various brain regions.

  6. Thermal neutron scattering data for 7LiF and BeF2

    NASA Astrophysics Data System (ADS)

    Wang, Jia; Song, Hongzhou; Hu, Zehua; Ye, Tao; Sun, Weili

    2017-09-01

    Based on the coherent elastic, incoherent elastic, coherent inelastic and incoherent inelastic scattering processes, a code named SIRIUS is developed to produce thermal neutron scattering data for crystals in ENDF-6 format. The phonon band structures and projected phonon densities of states of 7LiF and BeF2 crystals were calculated by Hellman-Feynman Theorem combined with a lattice dynamics direct method. Finally the thermal neutron scattering data for 7LiF and BeF2 crystals are given.

  7. Report for in-situ 7Li NMR experiment in PNNL Phase -1

    SciTech Connect

    Hu, Jian Zhi

    2014-08-19

    To understand the detailed local structural evolution, an in-situ 7Li NMR study was performed. An operando identification of the lithium germanide phases under various cycling regimens permitted understanding of the kinetics of phase transition between different structural phases, including the amorphous phases, and how these correlated with capacity retention. Combining data from TEM and in-situ 7Li NMR, we discovered that the phase inter-conversion during cycling was mediated by co-existing amorphous and crystalline phases, and that the high capacity observed was correlated with an over-lithiated lithium germanide phase.

  8. The energy spectrum of neutrons from 7Li(d,n)8Be reaction at deuteron energy 2.9 MeV

    NASA Astrophysics Data System (ADS)

    Mitrofanov, Konstantin V.; Piksaikin, Vladimir M.; Zolotarev, Konstantin I.; Egorov, Andrey S.; Gremyachkin, Dmitrii E.

    2017-09-01

    The neutron beams generated at the electrostatic accelerators using nuclear reactions T(p,n)3He, D(d,n)3He, 7Li(p,n)7Be, T(d,n)4He, 7Li(d,n)8Be, 9Be(d,n)10B are widely used in neutron physics and in many practical applications. Among these reactions the least studied reactions are 7Li(d,n)8Be and 9Be(d,n)10B. The present work is devoted to the measurement of the neutron spectrum from 7Li(d,n)8Be reaction at 0∘ angle to the deuteron beam axis on the electrostatic accelerator Tandetron (JSC "SSC RF - IPPE") using activation method and a stilbene crystal scintillation detector. The first time ever 7Li(d,n)8Be reaction was measured by activation method. The target was a thick lithium layer on metallic backing. The energy of the incident deuteron was 2.9 MeV. As activation detectors a wide range of nuclear reactions were used: 27Al(n,p)27Mg, 27Al(n,α)24Na, 113In(n,n')113mIn, 115In(n,n')115mIn, 115In(n,γ)116mIn, 58Ni(n,p)58mCo, 58Ni(n,2n)57Ni, 197Au(n,γ)198Au, 197Au(n,2n)196Au, 59Co(n,p)59Fe, 59Co(n,2n)58m+gCo, 59Co (n,g)60Co. Measurement of the induced gamma-activity was carried out using HPGe detector Canberra GX5019 [1]. The up-to-date evaluations of the cross sections for these reactions were used in processing of the data. The program STAYSL was used to unfold the energy spectra. The neutron spectra obtained by activation detectors is consistent with the corresponding data measured by a stilbene crystal scintillation detector within their uncertainties.

  9. A Monte Carlo dosimetry-based evaluation of the 7Li(p,n)7Be reaction near threshold for accelerator boron neutron capture therapy.

    PubMed

    Lee, C L; Zhou, X L; Kudchadker, R J; Harmon, F; Harker, Y D

    2000-01-01

    Advanced methods of boron neutron capture therapy (BNCT) use an epithermal neutron beam in conjunction with tumor-targeting boron compounds for irradiation of glioblastomas and metastatic melanomas. A common neutron-producing reaction considered for accelerator-based BNCT is 7Li(p,n)7Be, whose cross section increases very rapidly within several tens of keV of the reaction threshold at 1.88 MeV. Operation in the proton energy region near threshold will have an appreciable thick target neutron yield, but the neutrons produced will have relatively low energies that require little moderation to reach the epithermal range desirable for BNCT. Because of its relatively low projected accelerator cost and the portability of the neutron source/target assembly, BNCT based on the near-threshold technique is considered an attractive candidate for widespread hospital use. A systematic Monte Carlo N-Particle (MCNP) investigation of the dosimetric properties of near-threshold neutron beams has been performed. Results of these studies indicate that accelerator proton energies between 1.93 and 1.99 MeV, using 5 cm of H2O moderator followed by thin 6Li and Pb shields, can provide therapeutically useful beams with treatment times less than one hour and accelerator currents less than 5 mA.

  10. Thermal neutron detection using a silicon pad detector and {sup 6}LiF removable converters

    SciTech Connect

    Barbagallo, Massimo; Cosentino, Luigi; Marchetta, Carmelo; Pappalardo, Alfio; Scire, Carlotta; Scire, Sergio; Schillaci, Maria; Vecchio, Gianfranco; Finocchiaro, Paolo; Forcina, Vittorio; Peerani, Paolo; Vaccaro, Stefano

    2013-03-15

    A semiconductor detector coupled with a neutron converter is a good candidate for neutron detection, especially for its compactness and reliability if compared with other devices, such as {sup 3}He tubes, even though its intrinsic efficiency is rather lower. In this paper we show a neutron detector design consisting of a 3 cm Multiplication-Sign 3 cm silicon pad detector coupled with one or two external {sup 6}LiF layers, enriched in {sup 6}Li at 95%, placed in contact with the Si active surfaces. This prototype, first characterized and tested at INFN Laboratori Nazionali del Sud and then at JRC Ispra, was successfully shown to detect thermal neutrons with the expected efficiency and an outstanding gamma rejection capability.

  11. Sub-barrier fusion of weakly bound 6Li with 58Ni

    NASA Astrophysics Data System (ADS)

    Aguilera, E. F.; Martinez-Quiroz, E.; Amador-Valenzuela, P.; Lizcano, D.; García-Flores, A.; Kolata, J. J.; Roberts, A.; Rogachev, G. V.; Peaslee, G. F.; Guimarães, V.; Becchetti, F. D.; Villano, A.; Ojaruega, M.; Chen, Y.; Jiang, H.; Febbraro, M.; DeYoung, P. A.; Belyaeva, T. L.

    2017-08-01

    Evaporation-proton yields were measured for the fusion of the weakly bound nucleus 6Li on a 58Ni target at six near- or sub-barrier bombarding energies. Effects of the one-neutron transfer reaction were estimated and corrections made. Total-fusion cross sections were deduced using calculated proton multiplicities. The resulting fusion excitation function shows a considerable enhancement with respect to calculations for a bare potential. Inelastic couplings are estimated to have insignificant effects on such fusion. The sum of total fusion plus one-neutron transfer cross sections nearly saturates the total reaction cross section in the energy region measured. Comparison with previous results appropriately scaled for the 6Li+(59Co , 64Ni, 64Zn) systems shows good consistency except for some data spread at the lower energies.

  12. Scintillation properties of semiconducting 6LiInSe2 crystals to ionizing radiation

    NASA Astrophysics Data System (ADS)

    Wiggins, Brenden; Groza, Michael; Tupitsyn, Eugene; Lukosi, Eric; Stassun, Keivan; Burger, Arnold; Stowe, Ashley

    2015-11-01

    6LiInSe2 has gained attention recently as a semiconducting thermal neutron detector. As presented herein, the chalcogenide compound semiconductor also detects incident neutrons via scintillation, making 6LiInSe2 the only lithium containing semiconductor to respond to neutrons via both detection mechanisms. Both yellow and red crystals, which appear in the literature, were investigated. Only the yellow crystal responded favorably to ionizing radiation, similar to the semiconducting operation utilizing electrodes. The obtained light yield for yellow crystals is 4400 photons/MeV, referenced to Bi4Ge3O12 (BGO).The estimated thermal neutron light yield was 21,000 photons/thermal neutron. The two measured decay time components were found to be 31±1 ns (49%) and 143±9 ns (51%).This crystal provides efficient, robust detection of neutrons via scintillation with respectable light yield and rapid response, enabling its use for a broad array of neutron detection applications.

  13. First Tests of 6Li Doped Glass Scintillators for Ultracold Neutron Detection

    PubMed Central

    Ban, G.; Fléchard, X.; Labalme, M.; Lefort, T.; Liénard, E.; Naviliat-Cuncic, O.; Fierlinger, P.; Kirch, K.; Bodek, K.; Geltenbort, P.

    2005-01-01

    We report the results of test measurements aimed at determining the performances of 6Li doped glass scintillators for the detection of ultra-cold neutrons. Four types of scintillators, GS1, GS3, GS10 and GS20, which differ by their 6Li concentrations, have been tested. The signal to background separation is fully acceptable. The relative detection efficiencies have been determined as a function of the neutron velocity. We find that GS10 has a higher efficiency than the others for the detection of neutrons with velocities below 7 m/s. Two pieces of scintillators have been irradiated with a high flux of cold neutrons to test the radiation hardness of the glasses. No reduction in the pulse height has been observed up to an absorbed neutron dose of 1 × 1013 cm−3. PMID:27308137

  14. Giant resonances in {sup 116}Sn from 240 MeV {sup 6}Li scattering

    SciTech Connect

    Chen, X.; Lui, Y.-W.; Clark, H. L.; Tokimoto, Y.; Youngblood, D. H.

    2009-02-15

    Giant resonances in {sup 116}Sn were measured by inelastic scattering of {sup 6}Li ions at E{sub {sup 6}Li}=240 MeV over the angle range 0 deg. - 6 deg. Isoscalar E0-E3 strength distributions were obtained with a double folding model analysis. A total of 106{sub -11}{sup +27}% of the E0 EWSR was found in the excitation energy range from 8 MeV to 30 MeV with a centroid (m{sub 1}/m{sub 0}) energy 15.39{sub -0.20}{sup +0.35} MeV in agreement with results obtained with {alpha} inelastic scattering.

  15. Elastic Scattering and Fusion of {sup 6}Li on {sup 64}Zn at the Barrier

    SciTech Connect

    Scuderi, V.; Strano, E.; Amorini, F.; Lattuada, M.; Musumarra, A.; Pellegriti, M. G.; Rizzo, F.; Torresi, D.; Di Pietro, A.; Figuera, P.; Fisichella, M.; Maiolino, C.; Santonocito, D.; Goryunov, O.; Ostashko, V.; Papa, M.; Zadro, M.

    2011-10-28

    Elastic-scattering angular distributions for the {sup 6}Li+{sup 64}Zn system were measured at energies from below to above the Coulomb barrier. The experimental data were analyzed within the optical model to study the energy dependence of the interaction potential. The results suggest the presence of the breakup threshold anomaly. Preliminary results on the fusion cross-sections for the same system are also reported.

  16. Predicted isotopic variation in surface α clustering in Sn compared with (d ,6Li ) pickup yields

    NASA Astrophysics Data System (ADS)

    Cowley, A. A.

    2016-05-01

    Based on a generalized relativistic mean-field model, α clustering on the surface of Sn was recently predicted to vary systematically as a function of isotopic mass. Existing experimental information from (d ,6Li ) cluster pickup is now used to verify the predicted trend. The extent of the anticipated validity of such a comparison between the experimental results and the theoretical formulation is evaluated and discussed in the present paper.

  17. Barrier distributions for the {sup 7}Li+{sup 27}Al reaction

    SciTech Connect

    Cardenas, W. H. Z.

    2010-08-04

    Barrier distributions can be obtained from the first derivative of the elastic and quasielastic (QEL) backward angle excitation functions [1]. In this work we present a study of the barrier distribution for the {sup 7}Li+{sup 27}Al reaction from a Coupled-Channels Born Approximation (CCBA) calculations using the code FRESCO [2].

  18. Quasi-elastic pn scattering in 6LiD and 6LiH targets from 1.1 to 2.4 GeV

    NASA Astrophysics Data System (ADS)

    de Lesquen, A.; Allgower, C. E.; Ball, J.; Beddo, M.; Bystrický, J.; Combet, M.; Demierre, Ph.; Durand, G.; Fontaine, J.-M.; Grosnick, D.; Hess, R.; Janout, Z.; Janout, Z. F.; Kalinnikov, V. A.; Kasprzyk, T. E.; Khachaturov, B. A.; Kunne, R.; Lehar, F.; Lopiano, D.; Matafonov, V. N.; Pisarev, I. L.; Popov, A. A.; Prokofiev, A. N.; Rapin, D.; Sans, J.-L.; Spinka, H. M.; Usov, Yu. A.; Vikhrov, V. V.; Vuaridel, B.; Zhdanov, A. A.

    1999-11-01

    A polarized proton beam from SATURNE II, the Saclay polarized targets with ^6Li compounds, and an unpolarized CH_2 target were used to measure spin-dependent observables for protons scattered on bound nucleons. The beam and target polarizations were oriented vertically. The analyzing power A_{oono} and the depolarization D_{nono} were determined at seven energies between 1.1 and 2.4 GeV. The spin correlation parameter A_{oonn} was measured at only 1.1 and 1.6 GeV. Measurements with the CH_2 target at 1.1 GeV provided A_{oono} data for scattering of polarized protons on neutrons in carbon. The quasi-elastic observables are compared with previous elastic scattering measurements and at 1.1 GeV with predictions of phase shift analyses.

  19. Data for the neutron interactions with /sup 6/Li and /sup 10/B

    SciTech Connect

    Poenitz, W.P.

    1984-01-01

    The /sup 10/B(n,..cap alpha..), /sup 10/B(n,..cap alpha../sub 1/) and, increasingly in more recent measurement, the /sup 6/Li(n,..cap alpha..) cross sections are the major references used in low energy experiments. Many data from modern measurements are available for the neutron interaction with /sup 6/Li, including total, scattering, and absolute and relative (n,..cap alpha..) cross sections. A consensus has been reached with these new /sup 6/Li + n data. In contrast, the data base for the /sup 10/B neutron interaction cross sections is unfortunately poor. This is even the case for the total cross section which is supposed to be the easiest quantity to be measured. The most serious deficiency is the absence of data from absolute measurements of the /sup 10/B(n,..cap alpha..) and /sup 10/B(n,..cap alpha../sub 1/) cross sections in the last 10 to 15 years. The available cross section data which were used for the ENDF/B-VI evaluation will be discussed. 43 references.

  20. Effect of breakup and resonance states of6Li on fusion

    NASA Astrophysics Data System (ADS)

    Gómez Camacho, A.

    2017-07-01

    CDCC calculations of total fusion cross sections are presented for reactions of the weakly bound6Li with targets144Sm and154Sm at energies around the Coulomb barrier. Couplings to the low-lying excited states 2+, 3- of144Sm and 2+, 4+ of154Sm are included in the calculations. In the cluster structure frame of6Li → α + d, short range absorption potentials are considered for the interactions between α- and d- with the target to account for fusion. The effect of the excited states of the target on total fusion is investigated, as well as, that from couplings of resonance states of6Li, namely, l = 2, Jπ = 3+, 2+, 1+. The latter effect is calculated by two different approaches, (a) by considering only resonance states couplings and (b) by omitting these states from the full discretized energy space. Among other things, it is found that resonance and non-resonance continuum couplings give rise to small and similar fusion suppression at the higher energies.

  1. Barrier distribution functions for the system 6Li+64Ni and the effect of channel coupling

    NASA Astrophysics Data System (ADS)

    Shaikh, Md. Moin; Roy, Subinit; Rajbanshi, S.; Pradhan, M. K.; Mukherjee, A.; Basu, P.; Pal, S.; Nanal, V.; Pillay, R. G.; Shrivastava, A.

    2015-03-01

    Background: The barrier distribution function is an important observable in low-energy nucleus-nucleus collisions because it carries the distinct signature of the channel-coupling effect that is dominant at low energies. It can be derived from the fusion excitation function as well as from the back-angle quasi-elastic excitation function. The barrier distribution functions derived from the two complimentary measurements, in general, appear to peak at an energy close to the Coulomb barrier for strongly bound systems. But for weakly bound projectiles, like 6Li, a relative shift is observed between the distributions. Purpose: The present work investigates the barrier distribution functions from fusion as well as from the back-angle quasi-elastic excitation function for the 6Li+64Ni system. The purpose is to look for the existence of a shift, if any, between the two measured distribution functions, as reported for 6Li collision with heavy targets. A detailed coupled-channel calculation to probe the behavior of the distribution functions and their relative shift has been attempted. Measurement: A simultaneous measurement of fusion and back-angle quasi-elastic excitation functions for the system 6Li+64Ni was performed. The fusion excitation function was measured for the energy range of 11 to 28 MeV while the quasi-elastic excitation function measurement extended from 11 to 20 MeV. The barrier distribution functions were subsequently extracted from both the excitation functions and compared. Results: A small shift of around 450 keV peak to peak is observed between the barrier distribution functions derived from the complementary measurements. Detailed coupled channel and coupled reaction channel calculations reproduced both the excitation functions and barrier distributions. The shift of about 550 keV resulted from the model predictions corroborate the experimentally observed value for 6Li+64Ni system. Conclusions: The coupling to inelastic channels are found to be

  2. Unified description of ^{6}Li structure and deuterium-^{4}He dynamics with chiral two- and three-nucleon forces.

    PubMed

    Hupin, Guillaume; Quaglioni, Sofia; Navrátil, Petr

    2015-05-29

    We provide a unified ab initio description of the ^{6}Li ground state and elastic scattering of deuterium (d) on ^{4}He (α) using two- and three-nucleon forces from chiral effective field theory. We analyze the influence of the three-nucleon force and reveal the role of continuum degrees of freedom in shaping the low-lying spectrum of ^{6}Li. The calculation reproduces the empirical binding energy of ^{6}Li, yielding an asymptotic D- to S-state ratio of the ^{6}Li wave function in the d+α configuration of -0.027, in agreement with a determination from ^{6}Li-^{4}He elastic scattering, but overestimates the excitation energy of the 3^{+} state by 350 keV. The bulk of the computed differential cross section is in good agreement with data. These results endorse the application of the present approach to the evaluation of the ^{2}H(α,γ)^{6}Li radiative capture, responsible for the big-bang nucleosynthesis of ^{6}Li.

  3. Measurement of the differential cross sections of 6Li(d,d0) for Ion Beam Analysis purposes

    NASA Astrophysics Data System (ADS)

    Ntemou, E.; Aslanoglou, X.; Axiotis, M.; Foteinou, V.; Kokkoris, M.; Lagoyannis, A.; Misaelides, P.; Patronis, N.; Preketes-Sigalas, K.; Provatas, G.; Vlastou, R.

    2017-09-01

    In the present work, the 6Li(d,d0)6Li elastic scattering differential cross sections were measured in the energy range Ed,lab = 940-2000 keV for Elastic Backscattering Spectroscopy (EBS) purposes, using thin lithium targets, made by evaporating isotopically enriched 6LiF powder on self-supporting carbon foils, with an ultra-thin Au layer on top for normalization purposes. The experiment was carried out in deuteron beam energy steps of 20 or 30 keV and for the laboratory scattering angles of 125°, 140°, 150°, 160°, and 170°.

  4. Pole approximation validation in the study of the {sup 6}Li(d,{alpha}){sup 4}He reaction

    SciTech Connect

    Pizzone, R. G.; Kiss, G. G.; Spitaleri, C.; Lamia, L.; Cherubini, S.; La Cognata, M.; Puglia, S. M. R.; Rapisarda, G. G.; Romano, S.; Sergi, M. L.; Burjan, V.; Hons, Z.; Kroha, V.; Mrazek, J.; Piskor, S.; Li, C.; Tumino, A.

    2010-11-24

    The Trojan Horse Method (THM) was applied to the {sup 3}He+{sup 6}Li interaction in order to investigate the quasi-free {sup 6}Li(d,{alpha}){sup 4}He reaction. The experiment was performed at 17 MeV at the Cyclotron Institute of the Czech Academy of Science. The extracted {sup 6}Li(d,{alpha}){sup 4}He quasi-free cross-section was compared with the behavior of direct data. A good agreement between data sets shows up throughout the energy range investigated, providing a very important validity test of the pole approximation for the THM above the Coulomb barrier.

  5. Excitation function shape and neutron spectrum of the 7Li(p ,n )7Be reaction near threshold

    NASA Astrophysics Data System (ADS)

    Martín-Hernández, Guido; Mastinu, Pierfrancesco; Maggiore, Mario; Pranovi, Lorenzo; Prete, Gianfranco; Praena, Javier; Capote-Noy, Roberto; Gramegna, Fabiana; Lombardi, Augusto; Maran, Luca; Scian, Carlo; Munaron, Enrico

    2016-09-01

    The forward-emitted low energy tail of the neutron spectrum generated by the 7Li(p ,n )7Be reaction on a thick target at a proton energy of 1893.6 keV was measured by time-of-flight spectroscopy. The measurement was performed at BELINA (Beam Line for Nuclear Astrophysics) of the Laboratori Nazionali di Legnaro. Using the reaction kinematics and the proton on lithium stopping power the shape of the excitation function is calculated from the measured neutron spectrum. Good agreement with two reported measurements was found. Our data, along with the previous measurements, are well reproduced by the Breit-Wigner single-resonance formula for s -wave particles. The differential yield of the reaction is calculated and the widely used neutron spectrum at a proton energy of 1912 keV was reproduced. Possible causes regarding part of the 6.5% discrepancy between the 197Au(n ,γ ) cross section measured at this energy by Ratynski and Kappeler [Phys. Rev. C 37, 595 (1988), 10.1103/PhysRevC.37.595] and the one obtained using the Evaluated Nuclear Data File version B-VII.1 are given.

  6. Neutron total and scattering cross sections of /sup 6/Li in the few MeV region

    SciTech Connect

    Smith, A.; Guenther, P.; Whalen, J.

    1980-02-01

    Neutron total cross sections of /sup 6/Li are measured from approx. 0.5 to approx. 4.8 MeV at intervals of approx.< 10 keV. Neutron differential elastic-scattering cross sections are measured from 1.5 to 4.0 MeV at approx.> 10 scattering angles and at incident-neutron intervals of approx.< 100 keV. Neutron differential inelastic-scattering cross sections are measured in the incident-energy range 3.5 to 4.0 MeV. The experimental results are extended to lower energies using measured neutron total cross sections recently reported elsewhere by the authors. The composite experimental data (total cross sections from 0.1 to 4.8 MeV and scattering cross sections from 0.22 to 4.0 MeV) are interpreted in terms of a simple two-level R-matrix model which describes the observed cross sections and implies the reaction cross section in unobserved channels; notably the (n;..cap alpha..)t reaction (Q = 4.783 MeV). The experimental and calculational results are compared with previously reported results as summarized in the ENDF/B-V evaluated nuclear data file.

  7. Coupled channel effect in elastic scattering and fusion for 6,7Li+28Si

    NASA Astrophysics Data System (ADS)

    Sinha, Mandira; Roy, Subinit; Basu, P.; Majumdar, H.; Santra, S.; Parkar, V. V.; Golda, K. S.; Kailas, S.

    2011-10-01

    The fusion excitation and elastic angular distribution were measured for 6,7Li+28Si from below to above Coulomb barrier (≤ 3Vb) energies. The barrier distribution derived from the fusion data was found to be broad and asymmetric at the sub-barrier region, compared to 1D BPM estimation. Effect of rotational coupling on fusion was found to be not so dominant. Phenomenological optical potential parameters, with surface and volume type imaginary potentials, were obtained from f tting of elastic scattering data and energy dependence of real and imaginary surface strengths were investigated around the barrier. CDCC calculations considering only breakup of projectile were performed for 6,7Li+28Si with the elastic scattering data, using the code FRESCO. The effects of breakup of projectile on elastic cross section do not agree with the energy dependence of real and imaginary strength with volume type imaginary potential around the barrier.

  8. Role of the cluster structure of 7Li in the dynamics of fragment capture

    NASA Astrophysics Data System (ADS)

    Shrivastava, A.; Navin, A.; Diaz-Torres, A.; Nanal, V.; Ramachandran, K.; Rejmund, M.; Bhattacharyya, S.; Chatterjee, A.; Kailas, S.; Lemasson, A.; Palit, R.; Parkar, V. V.; Pillay, R. G.; Rout, P. C.; Sawant, Y.

    2013-01-01

    Exclusive measurements of prompt γ-rays from the heavy-residues with various light charged particles in the 7Li + 198Pt system, at an energy near the Coulomb barrier (E /Vb ∼ 1.6) are reported. Recent dynamic classical trajectory calculations, constrained by the measured fusion, α- and t-capture cross-sections have been used to explain the excitation energy dependence of the residue cross-sections. These calculations distinctly illustrate a two-step process, breakup followed by fusion, in case of the capture of t and α clusters; whereas for 6He + p and 5He + d configurations, massive transfer is inferred to be the dominant mechanism. The present work clearly demonstrates the role played by the cluster structures of 7Li in understanding the reaction dynamics at energies around the Coulomb barrier.

  9. A spectroscopic study of the 3(1) pi g Rydberg state of 7Li2.

    PubMed

    Song, Min; Yi, Peng; Dai, Xing-can; Liu, Yao-ming; Li, Li

    2002-06-01

    With pulsed optical-optical double resonance (OODR) fluorescence excitation spectroscopy Rydberg states of 7Li2 in the energy region of 35,500-38,000 cm-1 were studied and 146 transitions into the 3(1) pi g state of 7Li2 were measured. They were assigned to 10 vibrational levels of the 3(1) pi g state. A new set of Dunham constants, RKR potential curve, and Franck-Condon factors for the transitions form the A 1 sigma u+ state are derived. The perturbations between the 4(F)1 sigma g+, 5 (1) sigma g+, 6 (1) sigma g+, 2 (G) 1 pi g Rydberg states with the 3 (1) pi g state are discussed. The lambda-doubling splitting of the observed levels can be ignored with our accuracy (0.2 cm-1).

  10. Electric-field modulation of the magnetically induced 6Li-40K Feshbach resonance

    NASA Astrophysics Data System (ADS)

    Xie, Ting; Wang, Gao-Ren; Zhang, Wei; Huang, Yin; Cong, Shu-Lin

    2011-09-01

    The effect of an external electric field on the magnetically induced 6Li-40K Feshbach resonance is investigated theoretically by using the asymptotic bound state model (ABM). An electric field can modify the position and width of the Feshbach resonance to varying extent. However, it hardly changes the background scattering length in the case without open-channel resonance. The width of the s-wave resonance resulting from the p-wave bound state becomes narrow under the action of a strong electric field. The effects of electric field on orbital angular momentum and electronic state of the Feshbach molecule are also discussed.

  11. Study of silicon+6LiF thermal neutron detectors: GEANT4 simulations versus real data

    NASA Astrophysics Data System (ADS)

    Meo, S. Lo; Cosentino, L.; Mazzone, A.; Bartolomei, P.; Finocchiaro, P.

    2017-09-01

    Research and development on alternative thermal neutron detection technologies and methods are nowadays needed as a possible replacement of 3He-based ones. Commercial solid state silicon detectors, coupled with neutron converter layers containing 6Li, have been proved to represent a viable solution for several applications as present in the literature. In order to better understand the detailed operation and the response and efficiency of such detectors, a series of dedicated GEANT4 simulations were performed and compared with real data collected in a few different configurations. The results show an excellent agreement between data and simulations, indicating that the behavior of the detector is fully understood.

  12. Breakup threshold anomaly in the elastic scattering of {sup 6}Li on {sup 27}Al

    SciTech Connect

    Figueira, J. M.; Niello, J. O. Fernandez; Abriola, D.; Arazi, A.; Capurro, O. A.; Barbara, E. de; Marti, G. V.; Heimann, D. Martinez; Negri, A. E.; Pacheco, A. J.; Padron, I.; Gomes, P. R. S.; Lubian, J.; Correa, T.; Paes, B.

    2007-01-15

    Elastic scattering of the weakly bound {sup 6}Li on {sup 27}Al was measured at near-barrier energies. The data analysis was performed using a Woods-Saxon shape optical potential and also using the double-folding Sao Paulo potential. The results show the presence of the breakup threshold anomaly (BTA), an anomalous behavior when compared with the scattering of tightly bound nuclei. This behavior is attributed to a repulsive polarization potential produced by the coupling to the continuum breakup states.

  13. Repulsive Fermi Polarons in a Resonant Mixture of Ultracold 6Li Atoms

    NASA Astrophysics Data System (ADS)

    Scazza, F.; Valtolina, G.; Massignan, P.; Recati, A.; Amico, A.; Burchianti, A.; Fort, C.; Inguscio, M.; Zaccanti, M.; Roati, G.

    2017-02-01

    We employ radio-frequency spectroscopy to investigate a polarized spin mixture of ultracold 6Li atoms close to a broad Feshbach scattering resonance. Focusing on the regime of strong repulsive interactions, we observe well-defined coherent quasiparticles even for unitarity-limited interactions. We characterize the many-body system by extracting the key properties of repulsive Fermi polarons: the energy E+, the effective mass m*, the residue Z , and the decay rate Γ . Above a critical interaction, E+ is found to exceed the Fermi energy of the bath, while m* diverges and even turns negative, thereby indicating that the repulsive Fermi liquid state becomes energetically and thermodynamically unstable.

  14. Elastic scattering for the system {sup 6}Li+p at near barrier energies with MAGNEX

    SciTech Connect

    Soukeras, V.; Pakou, A.; Sgouros, O.; Cappuzzello, F.; Bondi, M.; Nicolosi, D.; Acosta, L.; Marquinez-Duran, G.; Martel, I.; Agodi, C.; Carbone, D.; Cavallaro, M.; Cunsolo, A.; Di Pietro, A.; Fernández-García, J. P.; Figuera, P.; Fisichella, M.; Alamanos, N.; De Napoli, M.; Foti, A.; and others

    2015-02-24

    Elastic scattering measurements have been performed for the {sup 6}Li+p system in inverse kinematics at the energies of 16, 20, 25 and 29 MeV. The heavy ejectile was detected by the large acceptance MAGNEX spectrometer at the Laboratori Nazionali del Sud (LNS) in Catania, in the angular range between ∼2{sup 0} and 12{sup 0} in the laboratory system, giving us the possibility to span almost a full angular range in the center of mass system. Results will be presented and discussed for one of the energies.

  15. Neutron detector based on Particles of 6Li glass scintillator dispersed in organic lightguide matrix

    NASA Astrophysics Data System (ADS)

    Ianakiev, K. D.; Hehlen, M. P.; Swinhoe, M. T.; Favalli, A.; Iliev, M. L.; Lin, T. C.; Bennett, B. L.; Barker, M. T.

    2015-06-01

    Most 3He replacement neutron detector technologies today have overlapping neutron-gamma pulse-height distributions, which limits their usefulness and performance. Different techniques are used to mitigate this shortcoming, including Pulse Shape Discrimination (PSD) or threshold settings that suppress all gammas as well as much of the neutrons. As a result, count rates are limited and dead times are high when PSD is used, and the detection efficiency for neutron events is reduced due to the high threshold. This is a problem in most applications where the neutron-gamma separation of 3He detectors had been essential. This challenge is especially severe for neutron coincidence and multiplicity measurements that have numerous conflicting requirements such as high detection efficiency, short die-away time, short dead time, and high stability. 6Li-glass scintillators have excellent light output and a single peak distribution, but they are difficult to implement because of their gamma sensitivity. The idea of reducing the gamma sensitivity of 6Li-glass scintillators by embedding small glass particles in an organic light-guide medium was first presented by L.M. Bollinger in the early 60s but, to the best of our knowledge, has never been reduced to practice. We present a proof of principle detector design and experimental data that develop this concept to a large-area neutron detector. This is achieved by using a multi-component optical medium (6Li glass particles attached to a glass supporting structure and a mineral oil light guide) which matches the indices of refraction and minimizes the absorption of the 395 nm scintillator light. The detector design comprises a 10 in. long tube with dual end readout with about 3% volume density of 6Li glass particles installed. The presented experimental data with various neutron and gamma sources show the desired wide gap between the neutron and gamma pulse height distributions, resulting in a true plateau in the counting

  16. Repulsive Fermi Polarons in a Resonant Mixture of Ultracold ^{6}Li Atoms.

    PubMed

    Scazza, F; Valtolina, G; Massignan, P; Recati, A; Amico, A; Burchianti, A; Fort, C; Inguscio, M; Zaccanti, M; Roati, G

    2017-02-24

    We employ radio-frequency spectroscopy to investigate a polarized spin mixture of ultracold ^{6}Li atoms close to a broad Feshbach scattering resonance. Focusing on the regime of strong repulsive interactions, we observe well-defined coherent quasiparticles even for unitarity-limited interactions. We characterize the many-body system by extracting the key properties of repulsive Fermi polarons: the energy E_{+}, the effective mass m^{*}, the residue Z, and the decay rate Γ. Above a critical interaction, E_{+} is found to exceed the Fermi energy of the bath, while m^{*} diverges and even turns negative, thereby indicating that the repulsive Fermi liquid state becomes energetically and thermodynamically unstable.

  17. Eu-doped 6LiF-SrF2 eutectic scintillators for neutron detection

    NASA Astrophysics Data System (ADS)

    Yanagida, Takayuki; Fukuda, Kentaro; Fujimoto, Yutaka; Kawaguchi, Noriaki; Kurosawa, Shunsuke; Yamazaki, Atsushi; Watanabe, Kenichi; Futami, Yoshisuke; Yokota, Yuui; Pejchal, Jan; Yoshikawa, Akira; Uritani, Akira; Iguchi, Tetsuo

    2012-03-01

    Eu2+ 0.05%, 0.1%, and 0.2% activated LiF-SrF2 eutectic scintillators were prepared by the Bridgman method using 6Li enriched (95%) raw material. The α-ray-induced radio luminescence spectra showed intense emission peak at 430 nm due to an emission from Eu2+ 5d-4f transition in the Eu:SrF2 layers. When excited by 252Cf neutrons, all the samples exhibited almost the same light yields of 5000-7000 ph/n with a typical decay times of several hundreds ns.

  18. New measurement of the 10B(n,α)7 Li through the Trojan Horse Method

    NASA Astrophysics Data System (ADS)

    Spartá, Roberta

    2016-04-01

    B(n,α) Li reaction cross section has been measured using the Trojan Horse method, with the specific aim to separate the α1 contribution (coming from the first Li excited level) by the αo (related to the Li ground state), using a very thin target. Preliminary results are shown of the three-body B(d,α7 Li)H cross section.

  19. Exploring Light Neutron Rich Nuclei via the ({sup 7}Li,{sup 7}Be) Reaction

    SciTech Connect

    Cavallaro, M.; Cappuzzello, F.; Cunsolo, A.; Foti, A.; Orrigo, S. E. A.; Rodrigues, M. R. D.; Borello-Lewin, T.; Lenske, H.; Petrascu, H.; Winfield, J. S.

    2008-11-11

    A systematic study of the nuclei that can be described as an integer number of {alpha} particles plus three neutrons via the ({sup 7}Li,{sup 7}Be) reaction at about 8 MeV/u has shown the presence of Bound States Embedded in the Continuum in the energy spectra. These are experimental signatures of the dynamical correlations of an easily polarizable core with a single-particle state of the valence neutron.

  20. Effects of distortion of the intercluster motion in {sup 2}H, {sup 3}He, {sup 3}H, {sup 6}Li, and {sup 9}Be on Trojan horse applications

    SciTech Connect

    Pizzone, R. G.; Spitaleri, C.; La Cognata, M.; Lamia, L.; Romano, S.; Mukhamedzhanov, A. M.; Blokhintsev, L. D.; Bertulani, C. A.; Irgaziev, B. F.

    2009-08-15

    Deuteron induced quasifree scattering and reactions have been extensively investigated in the past few decades as well as {sup 6}Li, {sup 3}H, {sup 3}He, and {sup 9}Be induced reactions. This was done not only for the investigation of nuclear structure and reaction mechanisms but also for important astrophysical applications (Trojan horse method). In particular the widths of the spectator momentum distributions in several nuclei, which have been used as Trojan horses, have been obtained as a function of the transferred momentum. Applications of Trojan horse method will also be discussed because the momentum distribution of the spectator particle inside the nucleus is a important input for this method. This gives hints on distortion effects at low energies important for nuclear astrophysics.

  1. Unified description of 6Li structure and deuterium-4He dynamics with chiral two- and three-nucleon forces

    DOE PAGES

    Hupin, Guillaume; Quaglioni, Sofia; Navratil, Petr

    2015-05-29

    Here, we provide a unified ab initio description of the 6Li ground state and elastic scattering of deuterium (d) on 4He (α) using two- and three-nucleon forces from chiral effective field theory. We analyze the influence of the three-nucleon force and reveal the role of continuum degrees of freedom in shaping the low-lying spectrum of 6Li. The calculation reproduces the empirical binding energy of 6Li, yielding an asymptotic D- to S-state ratio of the 6Li wave function in the d+α configuration of –0.027, in agreement with a determination from 6Li–4He elastic scattering, but overestimates the excitation energy of the 3+more » state by 350 keV. The bulk of the computed differential cross section is in good agreement with data. These results endorse the application of the present approach to the evaluation of the 2H(α,γ)6Li radiative capture, responsible for the big-bang nucleosynthesis of 6Li.« less

  2. Pulse-Shape Analysis of Neutron-Induced Scintillation Light in Ni-doped 6LiF/ZnS

    SciTech Connect

    Cowles, Christian C.; Behling, Richard S.; Imel, G. R.; Kouzes, Richard T.; Lintereur, Azaree; Robinson, Sean M.; Stave, Sean C.; Siciliano, Edward R.; Wang, Zheming

    2016-10-06

    Abstract–Alternatives to 3He are being investigated for gamma-ray insensitive neutron detection applications, including plutonium assay. One promising material is lithium-6 fluoride with silver activated zinc sulfide 6LiF/ZnS(Ag) in conjunction with a wavelength shifting plastic. Doping the 6LiF/ZnS(Ag) with nickel (Ni) has been proposed as a means of reducing the decay time of neutron signal pulses. This research performed a pulse shape comparison between Ni-doped and non-doped 6LiF/ZnS(Ag) neutron pulses. The Ni-doped 6LiF/ZnS(Ag) had a 32.7% ± 0.3 increase in neutron pulse height and a 32.4% ± 0.3 decrease in neutron pulse time compared to the non-doped 6LiF/ZnS(Ag). Doping 6LiF/ZnS(Ag) with nickel may allow neutron detector operation with improved signal to noise ratios, and reduced pulse pileup affects, increasing the accuracy and range of source activities with which such a detector could operate.

  3. Lifetime of Feshbach dimers in a Fermi-Fermi mixture of 6Li and 40K

    NASA Astrophysics Data System (ADS)

    Jag, M.; Cetina, M.; Lous, R. S.; Grimm, R.; Levinsen, J.; Petrov, D. S.

    2016-12-01

    We present a joint experimental and theoretical investigation of the lifetime of weakly bound dimers formed near narrow interspecies Feshbach resonances in mass-imbalanced Fermi-Fermi systems, considering the specific example of a mixture of 6Li and 40K atoms. Our work addresses the central question of the increase in the stability of the dimers resulting from Pauli suppression of collisional losses, which is a well-known effect in mass-balanced fermionic systems near broad resonances. We present measurements of the spontaneous dissociation of dimers in dilute samples, and of the collisional losses in dense samples arising from both dimer-dimer processes and from atom-dimer processes. We find that all loss processes are suppressed close to the Feshbach resonance. Our general theoretical approach for fermionic mixtures near narrow Feshbach resonances provides predictions for the suppression of collisional decay as a function of the detuning from resonance, and we find excellent agreement with the experimental benchmarks provided by our 40K-6Li system. We finally present model calculations for other Feshbach-resonant Fermi-Fermi systems, which are of interest for experiments in the near future.

  4. Optimizing ZnS/6LiF scintillators for wavelength-shifting-fiber neutron detectors

    SciTech Connect

    Crow, Lowell; Funk, Loren L; Hannan, Bruce W; Hodges, Jason P; Riedel, Richard A; Wang, Cai-Lin

    2016-01-01

    In this paper we compare the performance of grooved and flat ZnS/6LiF scintillators in a wavelength shifting-fiber (WLSF) detector. Flat ZnS/6LiF scintillators with the thickness L=0.2-0.8 mm were characterized using photon counting and pulse-height analysis and compared to a grooved scintillator of approximately 0.8 mm thick. While a grooved scintillator considerably increases the apparent thickness of the scintillator to neutrons for a given coating thickness, we find that the flat scintillators perform better than the grooved scintillators in terms of both light yield and neutron detection efficiency. The flat 0.8-mm-thick scintillator has the highest light output, and it is 52% higher compared with a grooved scintillator of same thickness. The lower light output of the grooved scintillator as compared to the flat scintillator is consistent with the greater scintillator-WLSF separation and the much larger average emission angle of the grooved scintillator. We also find that the average light cone width, or photon travel-length as measured using time-of-flight powder diffraction of diamond and vanadium, decreases with increasing L in the range of L=0.6-0.8 mm. This result contrasts with the traditional Swank diffusion model for micro-composite scintillators, and could be explained by a decrease in photon diffusion-coefficient or an increase in micro-particle content in the flat scintillator matrix for the thicker scintillators.

  5. Characterization of damage induced by heavy neutron irradiation on multilayered {sup 6}LiF-single crystal chemical vapor deposition diamond detectors

    SciTech Connect

    Almaviva, S.; Marinelli, Marco; Milani, E.; Prestopino, G.; Tucciarone, A.; Verona, C.; Verona-Rinati, G.; Angelone, M.; Pillon, M.

    2009-10-01

    the {sup 6}LiF layer has been found, the increased damage being ascribed to the highly ionizing particles produced in the {sup 6}LiF layer by thermal neutrons through the nuclear reaction {sup 6}Li(n,alpha)T.

  6. Central nervous system radiation syndrome in mice from preferential 10B(n, alpha)7Li irradiation of brain vasculature

    SciTech Connect

    Slatkin, D.N.; Stoner, R.D.; Rosander, K.M.; Kalef-Ezra, J.A.; Laissue, J.A.

    1988-06-01

    Ionizing radiations were directed at the heads of anesthetized mice in doses that evoked the acute central nervous system (CNS) radiation syndrome. Irradiations were done using either a predominantly thermal neutron field at a nuclear reactor after intraperitoneal injection of 10B-enriched boric acid or 250-kilovolt-peak x-rays with and without previous intraperitoneal injection of equivalent unenriched boric acid. Since 10B concentrations were approximately equal to 3-fold higher in blood than in cerebral parenchyma during the reactor irradiations, more radiation from alpha and 7Li particles was absorbed by brain endothelial cells than by brain parenchymal cells. Comparison of the LD50 dose for CNS radiation lethality from the reactor experiments with the LD50 dose from the x-ray experiments gives results compatible with morphologic evidence that endothelial cell damage is a major determinant of acute lethality from the CNS radiation syndrome. It was also observed that boric acid is a low linear energy transfer radiation-enhancement agent in vivo.

  7. A novel laser-collider used to produce monoenergetic 13.3 MeV 7Li (d, n) neutrons

    PubMed Central

    Zhao, J. R.; Zhang, X. P.; Yuan, D. W.; Li, Y. T.; Li, D. Z.; Rhee, Y. J.; Zhang, Z.; Li, F.; Zhu, B. J.; Li, Yan F.; Han, B.; Liu, C.; Ma, Y.; Li, Yi F.; Tao, M. Z.; Li, M. H.; Guo, X.; Huang, X. G.; Fu, S. Z.; Zhu, J. Q.; Zhao, G.; Chen, L. M.; Fu, C. B.; Zhang, J.

    2016-01-01

    Neutron energy is directly correlated with the energy of the incident ions in experiments involving laser-driven nuclear reactions. Using high-energy incident ions reduces the energy concentration of the generated neutrons. A novel “laser-collider” method was used at the Shenguang II laser facility to produce monoenergetic neutrons via 7Li (d, n) nuclear reactions. The specially designed K-shaped target significantly increased the numbers of incident d and Li ions at the keV level. Ultimately, 13.3 MeV neutrons were obtained. Considering the time resolution of the neutron detector, we demonstrated that the produced neutrons were monoenergetic. Interferometry and a Multi hydro-dynamics simulation confirmed the monoenergetic nature of these neutrons. PMID:27250660

  8. A novel laser-collider used to produce monoenergetic 13.3 MeV (7)Li (d, n) neutrons.

    PubMed

    Zhao, J R; Zhang, X P; Yuan, D W; Li, Y T; Li, D Z; Rhee, Y J; Zhang, Z; Li, F; Zhu, B J; Li, Yan F; Han, B; Liu, C; Ma, Y; Li, Yi F; Tao, M Z; Li, M H; Guo, X; Huang, X G; Fu, S Z; Zhu, J Q; Zhao, G; Chen, L M; Fu, C B; Zhang, J

    2016-06-02

    Neutron energy is directly correlated with the energy of the incident ions in experiments involving laser-driven nuclear reactions. Using high-energy incident ions reduces the energy concentration of the generated neutrons. A novel "laser-collider" method was used at the Shenguang II laser facility to produce monoenergetic neutrons via (7)Li (d, n) nuclear reactions. The specially designed K-shaped target significantly increased the numbers of incident d and Li ions at the keV level. Ultimately, 13.3 MeV neutrons were obtained. Considering the time resolution of the neutron detector, we demonstrated that the produced neutrons were monoenergetic. Interferometry and a Multi hydro-dynamics simulation confirmed the monoenergetic nature of these neutrons.

  9. A novel laser-collider used to produce monoenergetic 13.3 MeV 7Li (d, n) neutrons

    NASA Astrophysics Data System (ADS)

    Zhao, J. R.; Zhang, X. P.; Yuan, D. W.; Li, Y. T.; Li, D. Z.; Rhee, Y. J.; Zhang, Z.; Li, F.; Zhu, B. J.; Li, Yan F.; Han, B.; Liu, C.; Ma, Y.; Li, Yi F.; Tao, M. Z.; Li, M. H.; Guo, X.; Huang, X. G.; Fu, S. Z.; Zhu, J. Q.; Zhao, G.; Chen, L. M.; Fu, C. B.; Zhang, J.

    2016-06-01

    Neutron energy is directly correlated with the energy of the incident ions in experiments involving laser-driven nuclear reactions. Using high-energy incident ions reduces the energy concentration of the generated neutrons. A novel “laser-collider” method was used at the Shenguang II laser facility to produce monoenergetic neutrons via 7Li (d, n) nuclear reactions. The specially designed K-shaped target significantly increased the numbers of incident d and Li ions at the keV level. Ultimately, 13.3 MeV neutrons were obtained. Considering the time resolution of the neutron detector, we demonstrated that the produced neutrons were monoenergetic. Interferometry and a Multi hydro-dynamics simulation confirmed the monoenergetic nature of these neutrons.

  10. FIGARO : detecting nuclear materials using high-energy gamma rays for oxygen.

    SciTech Connect

    Michlich, B. J.; Smith, D. L.; Massey, T. N.; Ingram, D.; Fessler, A.

    2000-10-10

    Potential diversion of nuclear materials is a major international concern. Fissile (e.g., U, Pu) and other nuclear materials (e.g., D, Be) can be detected using 6-7 MeV gamma rays produced in the {sup 19}F(p,{alpha}{gamma}){sup 16}O reaction. These gamma rays will induce neutron emission via the photoneutron and photofission processes in nuclear materials. However, they are not energetic enough to generate significant numbers of neutrons from most common benign materials, thereby reducing the false alarm rate. Neutrons are counted using an array of BF3 counters in a polyethylene moderator. Experiments have shown a strong increase in neutron count rates for depleted uranium, Be, D{sub 2}O, and {sup 6}Li, and little or no increase for other materials (e.g., H{sub 2}O, SS, Cu, Al, C, {sup 7}Li). Gamma source measurements using solid targets of CaF{sub 2} and MgF{sub 2} and a SF{sub 6} gas target show that proton accelerator of 3 MeV and 10-100 microampere average current could lead to acceptable detection sensitivity.

  11. Studies of nuclear reaction at very low energies

    SciTech Connect

    Cecil, F.E.

    1992-01-15

    The deuteron radiative capture reactions on {sup 2}H, {sup 6}Li and {sup 10}B have been measured between center of mass energies of 20 and 140 keV. Of note is the observation that the gamma ray-to-charged particle branching ratio for the DD reaction appears independent of energy down to a center of mass energy of 20 keV, consistent with some and contrary to other theoretical models. We have investigated the ratio of the reactions D(d,p)T and D(d,n){sup 3}He down to c.m. energies of 3 keV and the ratio of the reactions 6Li(d,p){sup 7}Li and {sup 6}LI(d,{alpha}){sup 4}He down to a c.m. energy of 19 keV. The DD reaction ratio is independent of energy while the (d,p) branch of the D-{sup 6}Li evinces a significant enhancement at the lowest measured energies. We have continued our investigation of charged particle production from deuterium-metal systems at a modest level of activity. Noteworthy in this investigation is the observation of 3 MeV protons from deuteron beam loaded Ti and LiD targets subjected to extreme thermal disequilibria. Significant facility improvements were realized during the most recent contract period. Specifically the downstream magnetic analysis system proposed to eliminate beam induced contaminants has been installed and thoroughly tested. This improvement should allow the D(a,{gamma}){sup 6}Li reaction to be measured in the coming contract period. A scattering chamber required for the measurement of the {sup 7}Li({sup 3}He,p){sup 9}Be reaction has been designed, fabricated and installed on the accelerator. A CAMAC based charged particle identification system has been assembled also for use in our proposed measurement of the {sup 7}Li({sup 3}He, p){sup 9}Be.

  12. Time-of-flight calibration of a 6Li glass epithermal neutron detector

    PubMed

    Livingston; Saleh; Block; Brand

    2000-10-01

    The curing of Portland cement concrete involves the conversion of water from a free to a bound state. The process can be monitored nondestructively by measuring the shift in the neutron energy spectrum in the epithermal range (0.025-1 eV). A tuned array of 6Li glass detectors has been constructed with varying efficiencies over the epithermal energy range. To determine the efficiency of each detector as a function of neutron energy, it is necessary to calibrate it against a reference neutron spectrum. This was accomplished using a time-of-flight approach with a pulsed neutron beam produced at the Gaerttner LINAC Laboratory at Rensselaer Polytechnic Institute. With a neutron flight path of 25 m it was possible to determine the neutron detector efficiencies to an energy resolution of 11 microeV. The data showed good agreement with the detector design calculations.

  13. On the redistribution of 6Li+ ions implanted into polypropylene foils

    NASA Astrophysics Data System (ADS)

    Fink, D.; Behar, M.; Kaschny, J.; Klette, R.; Chadderton, L. T.; Hnatowicz, V.; Vacik, J.; Wang, L.

    1996-04-01

    6Li+ (150 keV) was implanted into thin polypropylene foils at fluences of 1 x 1013 to 1 x 1014 cm-2. Subsequent neutron depth profiling measurements of the Li distributions revealed considerable deviations from the expected ballistic range profiles. This Li redistribution was simulated by a numerical computer calculation. The best fit between measurements and simulations was obtained by assuming that ( i) Li redistributes immediately after its ballistic slowing-down, ( ii) the Li mobility is enhanced in the radiation-damaged polymer region, the local diffusion enhancement being controlled by the target's electronic damage, ( iii) mobile Li is readily trapped at radiation-induced defects, their density being proportional to the target's electronic damage, ( iv) these traps are saturable ones, and ( v) Li migration is not restricted to the ion track region, but proceeds also through the neighboring unirradiated bulk, though with slower speed.

  14. Fusion excitation function measurement for 6Li+64Ni at near-barrier energies

    NASA Astrophysics Data System (ADS)

    Moin Shaikh, Md.; Roy, Subinit; Rajbanshi, S.; Pradhan, M. K.; Mukherjee, A.; Basu, P.; Pal, S.; Nanal, V.; Pillay, R. G.; Shrivastav, A.

    2015-01-01

    Total fusion excitation function has been measured for the reaction of weakly bound 6Li projectile on medium mass 64Ni target at energies near the Coulomb barrier of the system. Online characteristic γ-ray detection method has been used to identify and determine the cross sections of the residues. No suppression of total fusion cross section (σTF) is observed at above barrier energies. But enhancement of measured cross section with respect to the one-dimensional barrier penetration model (1-DBPM) calculation is observed at below barrier energies. The enhancement can not be explained by coupled channels calculation with dominant projectile and target excitations as well as one-neutron stripping reaction.

  15. α-d resonances and the low-lying states of 6Li

    NASA Astrophysics Data System (ADS)

    Eskandarian, A.; Afnan, I. R.

    1992-12-01

    The low-lying states (below the 3-3H threshold) of the 6Li nucleus are generated using three-body models with two-body nonlocal separable interactions between the constituent particles. The positions and widths of the states are determined by searching for the eigenvalues of the kernel of the Faddeev equations in the complex energy plane. When appropriate (for T=0 states only), the results are compared with a separate determination of these quantities from the α-d scattering process. All experimentally observed levels are found. Given that the Coulomb interaction is not included in our calculations, agreement with experiment is favorable for both the positions and the widths of the resonances.

  16. Thermal neutron detection by entrapping 6LiF nanocrystals in siloxane scintillators

    NASA Astrophysics Data System (ADS)

    Carturan, S. M.; Marchi, T.; Maggioni, G.; Gramegna, F.; Degerlier, M.; Cinausero, M.; Dalla Palma, M.; Quaranta, A.

    2015-06-01

    Exploiting the long experience in design and production of scintillating mixtures based on siloxane matrices with combinations of primary dye and waveshifter, a first set of 6LiF loaded scintillator disks has been produced. The synthesis is herein described and reported, as well as preliminary results on their light response towards thermal neutrons. The preservation of transparency and mechanical integrity of the scintillator material is challenging when introducing the inorganic salt LiF which is a "foreign body" to the organic polysiloxane host matrix Different strategies such as synthesis of nanoparticles and surface functionalization have been pursued to succeed in the entrapment of the neutron converter whilst maintaining moderate light output, optical transparency and flexibility of the base scintillator.

  17. Elastic scattering of {sup 6}Li on {sup 64}Zn at near-barrier energies

    SciTech Connect

    Zadro, M.; Figuera, P.; Pietro, A. Di; Fisichella, M.; Maiolino, C.; Santonocito, D.; Amorini, F.; Lattuada, M.; Musumarra, A.; Pellegriti, M. G.; Rizzo, F.; Scuderi, V.; Torresi, D.; Goryunov, O.; Ostashko, V.; Papa, M.

    2009-12-15

    Elastic-scattering angular distributions for the {sup 6}Li+{sup 64}Zn system were measured at eight beam energies from below to above the Coulomb barrier, 12.0{<=}E{sub lab}{<=}22.0 MeV. The experimental data were analyzed within the optical model to study the energy dependence of the interaction potential and to obtain total reaction cross sections. The results obtained using several optical model potentials show similar behavior. The energy dependence of the strengths of the real and imaginary potentials suggests the presence of the breakup threshold anomaly. It is shown that the extracted energy dependence of the interaction potential at sub-barrier energies is very sensitive to possible experimental errors.

  18. Refractive versus resonant diffraction scattering of loosely bound 6Li nuclei

    NASA Astrophysics Data System (ADS)

    Carstoiu, Florin; Trache, Livius

    2012-05-01

    We present a complete analysis of 6Li+16O elastic scattering at 4 and 5 MeV/nucleon. Using either traditional Woods-Saxon or a range of semimicroscopic folding form factors we find that the data require deep, highly transparent potentials. Physically relevant solutions are selected according to the dispersion relation. The intermediate angle structures and the oscillatory increase of the cross section at large angles are interpreted either as a pre-rainbow oscillation resulting from the interference of the barrier and internal barrier far-side scattering subamplitudes or, equally well, as a resonant diffraction arising from two Regge poles located in peripheral waves. Both semiclassical and Regge pole approaches allow a dynamical separation of the resonant component of the S matrix.

  19. The 181Ta(7Li,5n)183Os reaction: Measurement and analysis of the excitation function and isomeric cross-section ratios

    NASA Astrophysics Data System (ADS)

    Ismail, M.; Sharma, R. P.; Rashid, M. H.

    1998-03-01

    Excitation function and isomeric cross-section ratios for the production of 183Osm,g by 7Li-induced reactions on 181Ta are obtained from the measurements of the residual activities by the conventional stacked-foils technique from threshold to 50 MeV. The excitation function and isomeric cross-section ratios for nuclear reaction 181Ta(7Li,5n)183Osm,g are compared with the theoretical statistical model calculation by using the ALICE/91, STAPRE, and CASCADE codes. In the energy range of the present measurement the excitation functions are fitted fairly well by both the geometry dependent hybrid (GDH) model and the hybrid model of Blann with initial exciton number n0=7 (nn=4, np=3, nh=0) using the ALICE/91 code. The experimental isomeric cross-section ratios are also reproduced fairly well by the calculation using the STAPRE code. However, the CASCADE code calculations slightly underpredict the cross section but reproduce the shape. In general, the statistical model under a suitable set of global assumptions, can reproduce the excitation function as well as isomeric cross-section ratios.

  20. Non-monotonic potentials and vector analyzing powers of 6,7Li scattering by 12C, 26Mg, 58Ni, and 120Sn

    NASA Astrophysics Data System (ADS)

    Basak, A. K.; Billah, M. M.; Kobra, M. J.; Sarkar, M. K.; Mizanur Rahman, M.; Das, Pretam K.; Hossain, S.; Abdullah, M. N. A.; Tariq, A. S. B.; Uddin, M. A.; Bhattacharjee, S.; Reichstein, I.; Malik, F. B.

    2011-06-01

    The data on the elastic scattering cross-section (CS) and vector analyzing power (VAP) of 6,7Li incident on 12C , 26Mg, 58Ni and 120Sn nuclei are analyzed in terms of an optical model (OM) potential, the real part of which is generated from a realistic two-nucleon interaction using the energy-density functional (EDF) formalism. The EDF-generated real part of the potential is non-monotonic (NM) in nature. This NM real potential part, without any renormalization, along with an empirically determined imaginary part and spin-orbit potential, embodying the underlying physics of projectile excitation, can successfully account for both CS and VAP data in all four cases. This investigation, for the first time, using the simple OM analysis accounts well for the opposite signs of the VAP data of elastically scattered 6,7Li by 58Ni at Elab≈20 MeV and by 120Sn at Elab=44 MeV. The ramification of successfully describing the data by the EDF-generated potential to the equation of state of nuclear matter is discussed.

  1. Novel 4π Detection System for the Measurement of the 6Li(n,α)3H Reaction Cross Section

    NASA Astrophysics Data System (ADS)

    Giorginis, Georgios; Bencardino, Raffaele

    2011-12-01

    A dedicated one-dimensional Time Projection Chamber (1D-TPC) was designed and produced at IRMM to determine the 6Li(n,α)3H cross section in the 0.4-2.8 MeV energy range, aiming at 5% accuracy. The basic TPC components were a twin gridded ionisation chamber (GIC) with interwired electrodes and fast digitisation of the anode and cathode signals. The energy of both reaction products emitted from a thin 6LiF sample at the common TPC cathode was measured. A Kr(97%)CO2(3%) mixture was used as the detector gas at a pressure up to 3.5 bar. A 238U sample mounted on the cathode of an ionisation chamber without grid was used as the neutron flux monitor. Special care was taken to reduce the experimental sources of uncertainty. The beam-monitor 238U sample was characterised at IRMM by low-geometry α-counting with an accuracy of 0.1%. A 6Li sample was produced at IRMM by vacuum evaporation of 6LiF onto transparent aluminium backing. The number of 6Li atoms will be measured via Thermal Neutron Depth Profiling with an expected accuracy of 2% with respect to an IRMM Standard Reference Material. First test measurements were performed using a monoenergetic neutron beam produced by the T(p,n)3He reaction at the IRMM 7 MV Van de Graaff accelerator. The experimental method and preliminary results are presented.

  2. Missing-mass spectroscopy with the 6Li(π-,K+)X reaction to search for H6Λ

    NASA Astrophysics Data System (ADS)

    Honda, R.; Agnello, M.; Ahn, J. K.; Ajimura, S.; Akazawa, Y.; Amano, N.; Aoki, K.; Bhang, H. C.; Chiga, N.; Endo, M.; Evtoukhovitch, P.; Feliciello, A.; Fujioka, H.; Fukuda, T.; Hasegawa, S.; Hayakawa, S. H.; Hosomi, K.; Hwang, S. H.; Ichikawa, Y.; Igarashi, Y.; Imai, K.; Ishibashi, N.; Iwasaki, R.; Joo, C. W.; Kiuchi, R.; Lee, J. K.; Lee, J. Y.; Matsuda, K.; Matsumoto, Y.; Matsuoka, K.; Miwa, K.; Mizoi, Y.; Moritsu, M.; Nagae, T.; Nagamiya, S.; Nakagawa, M.; Naruki, M.; Noumi, H.; Ota, R.; Roy, B. J.; Saha, P. K.; Sakaguchi, A.; Sako, H.; Samanta, C.; Samoilov, V.; Sasaki, Y.; Sato, S.; Sekimoto, M.; Shimizu, Y.; Shiozaki, T.; Shirotori, K.; Soyama, T.; Sugimura, H.; Takahashi, T.; Takahashi, T. N.; Tamura, H.; Tanabe, K.; Tanaka, T.; Tanida, K.; Tokiyasu, A. O.; Tsamalaidze, Z.; Ukai, M.; Yamamoto, T. O.; Yamamoto, Y.; Yang, S. B.; Yoshida, K.; J-PARC E10 Collaboration

    2017-07-01

    We searched for the bound state of the neutron-rich Λ -hypernucleus H6Λ, using the 6Li(π-,K+)X double charge-exchange reaction at a π- beam momentum of 1.2 GeV /c at J-PARC. A total of 1.4 ×1012π- was driven onto a 6Li target of 3.5-g /cm2 thickness. No event was observed below the bound threshold, i.e., the mass of H4Λ+2 n , in the missing-mass spectrum of the 6Li(π-,K+)X reaction in the 2∘<θπ K<20∘ angular range. Furthermore, no event was found up to 2.8 MeV /c2 above the bound threshold. We obtained the double-differential cross section spectra of the 6Li(π-,K+)X reaction in the angular range of 2∘<θπ K<14∘ . An upper limit of 0.56 nb/sr (90% C.L.) was obtained for the production cross section of the H6Λ hypernucleus bound state. In addition, not only the bound state region, but also the Λ continuum region and part of the Σ- quasifree production region of the 6Li(π-,K+ ) reaction were obtained with high statistics. The present missing-mass spectrum will facilitate the investigation of the Σ--nucleus optical potential for Σ--5He through spectrum shape analysis.

  3. Gamma-ray line emission from 7Li and 7Be production by cosmic-rays

    NASA Astrophysics Data System (ADS)

    Tatischeff, V.; Thibaud, J.-P.; Kiener, J.; Cassé, M.; Vangioni-Flam, E.

    2001-09-01

    We calculate the total γ-ray line emission at ~450 keV that accompanies 7Li and 7Be production by cosmic-ray interactions, including the delayed line emission at 0.478 MeV from 7Be radioactive decay. We present a new γ-ray spectroscopic test which has the potential to give direct information on the nature of the interstellar regions into which 7Be ions propagate and decay. Finally, we evaluate the intensity of the predicted diffuse emission from the central radian of the Galaxy.

  4. Beam shaping assembly optimization for (7)Li(p,n)(7)Be accelerator based BNCT.

    PubMed

    Minsky, D M; Kreiner, A J

    2014-06-01

    Within the framework of accelerator-based BNCT, a project to develop a folded Tandem-ElectroStatic-Quadrupole accelerator is under way at the Atomic Energy Commission of Argentina. The proposed accelerator is conceived to deliver a proton beam of 30mA at about 2.5MeV. In this work we explore a Beam Shaping Assembly (BSA) design based on the (7)Li(p,n)(7)Be neutron production reaction to obtain neutron beams to treat deep seated tumors.

  5. Revisiting the (7)Li(p,n)(7)Be reaction near threshold.

    PubMed

    Herrera, María S; Moreno, Gustavo A; Kreiner, Andrés J

    2014-06-01

    In this work we review all the available experimental neutron data for the (7)Li(p,n) reaction near threshold which is necessary to obtain an accurate source model for Monte Carlo simulations in Boron Neutron Capture Therapy. Scattered published experimental results such as cross sections, differential neutron yields and total yields were collected and analyzed, exploring the sensitivity of the fitting parameters to the different possible variables and deriving a consistent working set of parameters to evaluate the neutron source near threshold. Copyright © 2013 Elsevier Ltd. All rights reserved.

  6. Measurement of the parity-violating triton emission asymmetry in the reaction {sup 6}Li(n,{alpha}){sup 3}H with polarized cold neutrons

    SciTech Connect

    Vesna, V. A.; Shulgina, E. V.; Gledenov, Yu. M.; Sedyshev, P. V.; Nesvizhevsky, V. V.; Petoukhov, A. K.; Soldner, T.; Zimmer, O.

    2008-03-15

    We describe measurements of the parity-violating (P-odd) triton emission asymmetry coefficient a{sub P-odd} in the {sup 6}Li(n,{alpha}){sup 3}H reaction with polarized cold neutrons. Experiments were carried out at the Petersburg Nuclear Physics Institute (Gatchina, Russia) and at the Institut Laue-Langevin (Grenoble, France). We employed an ionisation chamber in a configuration allowing us to suppress the left-right asymmetry well below 10{sup -8}. An additional test for a false asymmetry due to eventual target impurities (''zero test'') resulted in a{sub 0-test}=(0.0{+-}0.5)x10{sup -8}. As final result of this series of experiments we obtained a{sub P-odd}=(-8.8{+-}2.1)x10{sup -8}.

  7. Cross sections and analyzing powers for (p ⃗,n p ) reactions of 2H, 6Li, and 12C at 296 MeV

    NASA Astrophysics Data System (ADS)

    Wakasa, T.; Yasuda, J.; Dozono, M.; Fukunaga, T.; Gotanda, S.; Hatanaka, K.; Ishibashi, K.; Kanaya, Y.; Kimura, S.; Maeda, Y.; Maeda, Y.; Nishio, Y.; Noro, T.; Nozoe, T.; Ohnaka, K.; Sakaguchi, S.; Sakemi, Y.; Sekiguchi, K.; Taguchi, T.; Wada, Y.

    2017-07-01

    We report measurements of cross sections and analyzing powers for nucleon-knockout (p ⃗,n p ) reactions of 2H, 6Li, and 12C at 296 MeV using the RCNP NPOL3 neutron detector and large acceptance spectrometer. The 1 s and 1 p knockout reactions were successfully separated with a separation-energy resolution of approximately 6 MeV. The resulting data were compared with plane-wave and distorted-wave impulse approximation calculations employing the nucleon-nucleon t matrix in free space. No significant differences were identified in the case of the present analyzing power data, in contrast to the significant reductions observed in (p ⃗,2 p ) values. The conventional Pauli blocking and nuclear binding effects with the g matrix and the relativistic effect of nucleon mass reduction in the nuclei are also discussed.

  8. Breakup of 6Li+p at near-barrier energies and the effect on elastic scattering

    NASA Astrophysics Data System (ADS)

    Soukeras, V.; Pakou, A.; Cappuzzello, F.; Acosta, L.; Agodi, C.; Alamanos, N.; Calabrese, S.; Carbone, D.; Cavallaro, M.; Cunsolo, A.; Di Pietro, A.; Fernández-García, J. P.; Figuera, P.; Fisichella, M.; Foti, A.; Keeley, N.; Marquınez-Duràn, G.; Martel, I.; Mazzocco, M.; Pierroutsakou, D.; Rusek, K.; Santagati, G.; Sgouros, O.; Stiliaris, E.; Strano, E.; Torresi, D.; Zerva, K.

    2017-05-01

    Exclusive breakup measurements have been performed for the 6Li+p system in inverse kinematics at 6Li incident energies of 25 and 29 MeV. The results are considered in the Continuum Discretized Coupled-Channels framework, together with elastic scattering data at 16, 20, 25, and 29 MeV, obtained simultaneously in the same experiment and reported previously. Good agreement between data and theory is observed, interpreted as evidence for strong coupling to the continuum. The direct and sequential (via the 6Li31+ resonance) breakup cross sections are found to be equally large at the higher incident energies but the dominant effect on the elastic scattering is due to coupling to the sequential breakup. This effect remains dominant even at the lowest energy of 16 MeV, despite the negligible cross section for excitation of the resonance at this low incident energy.

  9. Giant resonances in {sup 24}Mg and {sup 28}Si from 240 MeV {sup 6}Li scattering

    SciTech Connect

    Chen, X.; Lui, Y.-W.; Clark, H. L.; Tokimoto, Y.; Youngblood, D. H.

    2009-07-15

    Elastic and inelastic scattering of 240 MeV {sup 6}Li particles from {sup 24}Mg and {sup 28}Si were measured with the MDM spectrometer. Optical potential parameters for {sup 6}Li+{sup 24}Mg and {sup 6}Li+{sup 28}Si scattering systems were obtained by fitting elastic scattering with two different folding model potentials as well as W-S potentials. E0-E3 giant resonance strength distributions for {sup 28}Si and {sup 24}Mg were obtained. E0 strength corresponding to 106{sub -24}{sup +34}% of the EWSR was identified in {sup 24}Mg and 80{sub -20}{sup +35}% was found for {sup 28}Si between E{sub x}=8.0 to 40.0 MeV.

  10. Ab initio calculations of nuclear reactions important for astrophysics

    NASA Astrophysics Data System (ADS)

    Navratil, Petr; Dohet-Eraly, Jeremy; Calci, Angelo; Horiuchi, Wataru; Hupin, Guillaume; Quaglioni, Sofia

    2016-09-01

    In recent years, significant progress has been made in ab initio nuclear structure and reaction calculations based on input from QCD employing Hamiltonians constructed within chiral effective field theory. One of the newly developed approaches is the No-Core Shell Model with Continuum (NCSMC), capable of describing both bound and scattering states in light nuclei simultaneously. We will present NCSMC results for reactions important for astrophysics that are difficult to measure at relevant low energies, such as 3He(α,γ)7Be and 3H(α,γ)7Li and 11C(p,γ)12N radiative capture, as well as the 3H(d,n)4He fusion. We will also address prospects of calculating the 2H(α,γ)6Li capture reaction within the NCSMC formalism. Prepared in part by LLNL under Contract DE-AC52-07NA27344. Supported by the U.S. DOE, OS, NP, under Work Proposal No. SCW1158, and by the NSERC Grant No. SAPIN-2016-00033. TRIUMF receives funding from the NRC Canada.

  11. Corrosion barriers processed by Al electroplating and their resistance against flowing Pb-15.7Li

    NASA Astrophysics Data System (ADS)

    Krauss, Wolfgang; Konys, Jürgen; Wulf, Sven-Erik

    2014-12-01

    In the HCLL blanket design, ferritic-martensitic steels are in direct contact with the flowing liquid breeder Pb-15.7Li and have to withstand severe corrosion attack. Beyond corrosion, T-permeation from the breeder into the RAFM-steels is also an important issue and has to be reduced significantly. Earlier work showed that Al-based coatings can act as barriers for both, however, applied processes e.g. HDA or VPS exhibited strong drawbacks in the past. Meanwhile new industrial relevant coating processes, using electroplating technology are under development and called ECA (electrochemical aluminization) and ECX (electrochemical deposition from ionic liquids) process. In this study electrochemically Al-coated and heat-treated Eurofer samples were tested in PICOLO loop for exposure times up to 12,000 h (ECA) and 2000 h (first results ECX) respectively to determine corrosion properties in flowing Pb-15.7Li (550 °C, 0.1 m/s). Cross section analysis afterward corrosion testing proved the ability of thin Al-based barriers made by electrochemical techniques to protect the bare Eurofer from corrosion attack even at exposure times of 12,000 h. Determined radial corrosion rates lay between 10 and 20 μm/a. First results for ECX coated samples (2000 h) revealed more homogeneous corrosion behavior of the barrier layer itself compared to ECA.

  12. Astrophysical S factors for radiative proton capture by {sup 3}H and {sup 7}Li nuclei

    SciTech Connect

    Dubovichenko, S. B.

    2011-03-15

    Within the potential cluster model where orbital states are classified according to Young diagrams and isospin, astrophysical S factors are considered for radiative proton capture by {sup 3}H and {sup 7}Li nuclei at energies of up to 1 and 10 keV, respectively. It is shown that the approach used, which takes into account only the E1 transition for the p{sup 3}H capture process, makes it possible to describe well the most recent experimental data at c.m. energies in the range from 50 keV to 5MeV. In the case of proton capture by {sup 7}Li nuclei, an M1 processwas taken into account in addition to the E1 transition, and a general behavior and the magnitude of the experimental S factor could be correctly reproduced owing to this at astrophysical energies, including the region around the resonance at 0.441 MeV (in the laboratory frame).

  13. (7)Li in situ 1D NMR imaging of a lithium ion battery.

    PubMed

    Klamor, S; Zick, K; Oerther, T; Schappacher, F M; Winter, M; Brunklaus, G

    2015-02-14

    The spatial distribution of charge carriers in lithium ion batteries during current flow is of fundamental interest for a detailed understanding of transport properties and the development of strategies for future improvements of the electrolyte-electrode interface behaviour. In this work we explored the potential of (7)Li 1D in situ NMR imaging for the identification of concentration gradients under constant current load in a battery cell. An electrochemical cell based on PTFE body and a stack of glass microfiber discs that are soaked with a technically relevant electrolyte suitable for high-temperature application and squeezed between a Li metal and a nano-Si-graphite composite electrode was assembled to acquire (7)Li 1D in situ NMR profiles with an improved NMR pulse sequence as function of time and state of charge, thereby visualizing the course of ion concentration during charge and discharge. Surface localized changes of Li concentration were attributed to processes such as solid electrolyte interphase formation or full lithiation of the composite electrode. The method allows the extraction of lithium ion transport properties.

  14. Preparation of 6LiF deposits and characterisation via Monte Carlo simulations and Neutron Depth Profiling

    NASA Astrophysics Data System (ADS)

    Bencardino, R.; Giorginis, G.; Sapundjiev, D.

    2013-05-01

    The Institute for Reference Materials and Measurements (IRMM) is measuring the 6Li(n,t)4He cross-section aiming at extending its status of standard over the MeV energy range. We developed a protocol to stretch-mount 0.75 μm, 1.5 μm, 8 μm, and 20 μm thick aluminium foils onto 0.5 mm thick tantalum rings. 6LiF samples were produced depositing, by vacuum evaporation onto aluminium backings, a layer of lithium fluoride 95.5% enriched in 6Li. We engineered dedicated tools and containers to handle and transport the resulting samples. These were characterised first at IRMM by differential weighing, then by Neutron Depth Profiling (NDP) at the TU Delft. These two measurements were found to be consistent for a selected sample, probed by a thermal neutron beam in three different regions to measure the 6LiF layer thickness and uniformity (defined as variation of the thickness relative to its average). The latter was found to be 0.8%, and the 6Li thickness to be 7.30±0.12, 7.35±0.12, and 7.29±0.12 μg/cm2 in the three regions. We performed Monte Carlo simulations to estimate the uniformity of the 6LiF layer, and benchmarked the calculation against the NDP measurements. They were consistent with respect to the deposit uniformity although the simulations were found to overestimate the thickness of the layer.

  15. {sup 6}LiF:ZnS(Ag) Neutrons Scintillator Detector Configuration for Optimal Readout

    SciTech Connect

    Osovizky, A.; Yehuda-Zada, Y.; Ghelman, M.; Tsai, P.; Thompson, A.K.; Pritchard, K.; Ziegler, J.B.; Ibberson, R.M.; Majkrzak, C.F.; Maliszewskyj, N.C.

    2015-07-01

    A Chromatic Analysis Neutron Diffractometer Or Reflectometer (CANDOR) is under development at the NIST Center for Neutron Research (NCNR). The CANDOR neutron sensor will rely on scintillator material for detecting the neutrons scattered by the sample under test. It consists of {sup 6}LiF:ZnS(Ag) scintillator material into which wavelength shifting (WLS) fibers have been embedded. Solid state photo-sensors (silicon photomultipliers) coupled to the WLS fibers are used to detect the light produced by the neutron capture event ({sup 6}Li (n,α) {sup 3}H reaction) and ionization of the ZnS(Ag). This detector configuration has the potential to accomplish the CANDOR performance requirements for efficiency of 90% for 5 A (3.35 meV) neutrons with high gamma rejection (10{sup 7}) along with compact design, affordable cost and materials availability. However this novel design includes challenges for precise neutron detection. The recognizing of the neutron signature versus the noise event produce by gamma event cannot be easy overcome by pulse height discrimination obstacle as can be achieved with {sup 3}He gas tube. Furthermore the selection of silicon photomultipliers (SiPM) as the light sensor maintains the obstacle of dark noise that does not exist when a photomultiplier tube is coupled to the scintillator. A proper selection of SiPM should focus on increasing the output signal and reducing the dark noise in order to optimize the detection sensitivity and to provide a clean signal pulse shape discrimination. The main parameters for evaluation are: - Quantum Efficiency (QE) - matching the SiPM peak QE with the peak transmission wavelength emission of the WLS. - Recovery time - a short recovery time is preferred to minimize the pulse width beyond the intrinsic decay time of the scintillator crystal (improves the gamma rejection based output pulse shape (time)). - Diode dimensions -The dark noise is proportional to the diode active area while the signal is provided by the

  16. Projectile-breakup-induced fission-fragment angular distributions in the 6Li+232Th reaction

    NASA Astrophysics Data System (ADS)

    Pal, A.; Santra, S.; Chattopadhyay, D.; Kundu, A.; Ramachandran, K.; Tripathi, R.; Roy, B. J.; Nag, T. N.; Sawant, Y.; Sarkar, D.; Nayak, B. K.; Saxena, A.; Kailas, S.

    2017-08-01

    Background: Experimental anisotropy in fission-fragment (FF) angular distribution in reactions involving weakly bound stable projectiles with actinide targets are enhanced compared to statistical saddle-point model (SSPM) predictions. Contributions from breakup- or transfer-induced fission to total fission are cited as possible reasons for such enhancement. Purpose: To identify the breakup- or transfer-induced fission channels in 6Li+232Th reaction and to investigate their effects on FF angular anisotropy. Methods: The FF angular distributions have been measured exclusively at three beam energies (28, 32, and 36 MeV) around the Coulomb barrier in coincidence with projectile breakup fragments like α , d , and p using Si strip detectors. The angular anisotropy obtained for different exclusive breakup- or transfer-induced fission channels are compared with that for total fission. SSPM and pre-equilibrium fission models have been employed to obtain theoretical FF angular anisotropy. Results: Angular anisotropy of the fission fragments produced by different transfer- or breakup-induced fission reactions have been obtained separately in the rest frame of respective recoiling nuclei. Some of these anisotropies were found to be stronger than those of the inclusive fission. Overall angular distributions of transfer or breakup fission, integrated over all possible recoil angles with weight factor proportional to differential cross section of the complementary breakup fragment emitted in coincidence in all possible directions, were obtained. It was observed that the overall FF angular anisotropy for each of these fission channels is less than or equal to the anisotropy of total fission at all the measured energies. Assuming isotropic out-of-plane correlations between the fission fragments and light-charged particles, the overall breakup- or transfer-induced fission fragment angular distributions do not explain the observed enhancement in FF anisotropy of total fission. Pre

  17. Heterogeneous Coordination Environments in Lithium-Neutralized Ionomers Identified Using 1H and 7Li MAS NMR

    PubMed Central

    Alam, Todd M.; Jenkins, Janelle E.; Bolintineanu, Dan S.; Stevens, Mark J.; Frischknecht, Amalie L.; Buitrago, C. Francisco; Winey, Karen I.; Opper, Kathleen L.; Wagener, Kenneth B.

    2012-01-01

    The carboxylic acid proton and the lithium coordination environments for precise and random Li-neutralized polyethylene acrylic acid P(E-AA) ionomers were explored using high speed solid-state 1H and 7Li MAS NMR. While the 7Li NMR revealed only a single Li coordination environment, the chemical shift temperature variation was dependent on the precise or random nature of the P(E-AA) ionomer. The 1H MAS NMR revealed two different carboxylic acid proton environments in these materials. By utilizing 1H-7Li rotational echo double resonance (REDOR) MAS NMR experiments, it was demonstrated that the proton environments correspond to different average 1H-7Li distances, with the majority of the protonated carboxylic acids having a close through space contact with the Li. Molecular dynamics simulations suggest that the shortest 1H-7Li distance corresponds to un-neutralized carboxylic acids directly involved in the coordination environment of Li clusters. These solid-state NMR results show that heterogeneous structural motifs need to be included when developing descriptions of these ionomer materials.

  18. 7Li-induced reaction on natMo: A study of complete versus incomplete fusion

    NASA Astrophysics Data System (ADS)

    Kumar, Deepak; Maiti, Moumita; Lahiri, Susanta

    2017-07-01

    Background: Several investigations on the complete-incomplete fusion (CF-ICF) dynamics of α -cluster well-bound nuclei have been contemplated above the Coulomb barrier (˜4 -7 MeV/nucleon) in recent years. It is therefore expected to observe significant ICF over CF in the reactions induced by a weakly bound α -cluster nucleus at slightly above the barrier. Purpose: Study of the CF-ICF dynamics by measuring the populated residues in the weakly bound 7Li+natMo system at energies slightly above the Coulomb barrier to well above it. Method: In order to investigate CF-ICF in the loosely bound system, 7Li beam was bombarded on the natMo foils, separated by the aluminium (Al) catcher foils alternatively, within ˜3 -6.5 MeV/nucleon. Evaporation residues produced in each foil were identified by the off-line γ -ray spectrometry. Measured cross section data of the residues were compared with the theoretical model calculations based on the equilibrium (EQ) and pre-equilibrium (PEQ) reaction mechanisms. Results: The experimental cross section of Rh 101 m,100 ,99 m,97 ,Ru,9597,Tc 99 m,96 ,95 ,94 ,93 m+g , and 93mMo residues measured at various projectile energies were satisfactorily reproduced by the simplified coupled channel approach in comparison to single barrier penetration model calculation. Significant cross section enhancement in the α -emitting channels was observed compared to EQ and PEQ model calculations throughout observed energy region. The ICF process over CF was analyzed by comparing with EMPIRE. The increment of the incomplete fusion fraction was observed with increasing projectile energies. Conclusions: Theoretical model calculations reveal that the compound reaction mechanism is the major contributor to the production of residues in 7Li+natMo reaction. Theoretical evaluations substantiate the contribution of ICF over the CF in α -emitting channels. EMPIRE estimations shed light

  19. Two phase morphology limits lithium diffusion in TiO(2)(anatase): a (7)Li MAS NMR study.

    PubMed

    Wagemaker, M; van de Krol, R; Kentgens, A P; van Well, A A; Mulder, F M

    2001-11-21

    7Li magic angle spinning solid-state nuclear magnetic resonance is applied to investigate the lithium local environment and lithium ion mobility in tetragonal anatase TiO(2) and orthorhombic lithium titanate Li(0.6)TiO(2). Upon lithium insertion, an increasing fraction of the material changes its crystallographic structure from anatase TiO(2) to lithium titanate Li(0.6)TiO(2). Phase separation occurs, and as a result, the Li-rich lithium titanate phase is coexisting with the Li-poor TiO(2) phase containing only small Li amounts approximately equal to 0.01. In both the anatase and the lithium titanate lattice, Li is found to be hopping over the available sites with activation energies of 0.2 and 0.09 eV, respectively. This leads to rapid microscopic diffusion rates at room temperature (D(micr) = 4.7 x 10(-12) cm(2)s(-1) in anatase and D(micr) = 1.3 x 10(-11) cm(2)s(-1) in lithium titanate). However, macroscopic intercalation data show activation energies of approximately 0.5 eV and smaller diffusion coefficients. We suggest that the diffusion through the phase boundary is determining the activation energy of the overall diffusion and the overall diffusion rate itself. The chemical shift of lithium in anatase is independent of temperature up to approximately 250 K but decreases at higher temperatures, reflecting a change in the 3d conduction electron densities. The Li mobility becomes prominent from this same temperature showing that such electronic effects possibly facilitate the mobility.

  20. Characterization of a ^6Li-loaded organic liquid scintillator for fast neutron spectrometry

    NASA Astrophysics Data System (ADS)

    Bass, C. D.; Heimbach, C. R.; Nico, J. S.; Beise, E. J.; Breuer, H.; Erwin, D.; Langford, T.; Rodrigues, A.

    2010-11-01

    Fast neutrons induced by natural radioactivity and cosmic rays are important sources of background for low-background searches of dark matter, neutrinoless double beta decay, and solar neutrinos. One method for performing fast neutron spectroscopy involves a capture-gated coincidence between a fast neutron that thermalizes through elastic scattering within an organic scintillator and its subsequent capture on a nuclide having a high thermal neutron capture cross section. Thermalization within an organic scintillator occurs within a few ns, but the neutron capture time is typically of order 10s to 100s of μs. A capture signal preceded by a thermalization signal within a characteristic time can be used to select those fast neutrons that have deposited all of their kinetic energy into the scintillator, and the thermalization signal can provide spectroscopic information. We report on a number of measurements performed to characterize the properties of an organic liquid scintillator based on di-isopropyl naphthalene and loaded with ^6Li. This work has been carried out within a joint UMd and NIST project to develop a fast neutron spectrometer suitable for use in a deep underground, low-background laboratory. In particular, we report on measurements of optical properties, light yield, and fast neutron response.

  1. Development of a 6LiF/ZnS-based Neutron Multiplicity Counter

    SciTech Connect

    Stave, Sean C.; Behling, Richard S.; Bernacki, Bruce E.; Bliss, Mary; Cowles, Christian C.; Kouzes, Richard T.; Lintereur, Azaree; Robinson, Sean M.; Siciliano, Edward R.

    2016-10-06

    Abstract–Neutron multiplicity counters are used in safeguards to provide rapid assay of samples which contain an unknown amount of plutonium in a potentially unknown configuration. A project at PNNL is using regular and nickel-quenched 6LiF/ZnS neutron-scintillator sheets and wavelength shifting plastic for light pipes in place of 3He. A combination of laboratory and modeling work predicts a LiF/ZnS-based system to be able to match or exceed the performance of the best 3He-based systems available. Also, the Ni-quenched material is expected to allow for improved neutron/gamma-ray discrimination at twice the event rate relative to the non-Ni-quenched LiF/ZnS. A new system based on the LiF/ZnS material is under construction and components are being used to optimize the detection efficiency and neutron/gamma-ray discrimination properties. Components of the new system are partially constructed and undergoing performance testing utilizing high-speed digitizers with field programmable gate arrays to perform the neutron/gamma-ray discrimination. The expected performance of the full-scale system is expected to be nearly the same as for 3He-based systems and is due for completion in 2016.

  2. Damage profile examination on ion irradiated PEEK by 6Li doping and neutron depth profiling technique

    NASA Astrophysics Data System (ADS)

    Vacík, J.; Červená, J.; Hnatowicz, V.; Švorčík, V.; Kobayashi, Y.; Fink, D.; Klett, R.

    1998-05-01

    Depth structure of radiation damaged surface layer of poly(aryl-ether-ether ketone) (PEEK) a polymer was studied using doping with 6Li atoms combined with nondestructive neutron depth profiling (NDP) method. The PEEK foils were irradiated with 2 MeV O + ions up to a fluence of 6 × 10 14 ions/cm 2. The damage profiles in the samples were visualized by doping of the samples with 5 M LiCl water solution at room temperature (RT) for 22.5 h. The Li ions are trapped on ion-produced radiation defects and the Li depth profiles are determined by the NDP method. NDP experiments were performed before and after leaching of excess of lithium atoms from the samples in distilled water at RT for 2 h. The leaching leads to dramatic changes in the Li depth distribution which, at low ion fluences, is similar in shape to the electronic energy loss profile of 2 MeV O + ions. For the higher fluences double-peaked profile occurs, which indicates a competition between different degradation processes in ion irradiated polymer.

  3. Crystal growth and characterization of 6LiInSe2 neutron detector

    NASA Astrophysics Data System (ADS)

    Cui, Yunlong; Bhattacharya, Pijush; Groza, Michael; Tupitysn, Eugene; Rowe, Emmanuel; Buliga, Vladimir; Matei, Liviu; Wiggins, Brenden; Johnstone, Daniel; Stowe, Ashley; Burger, Arnold

    2014-03-01

    6LiInSe2 is a promising thermal neutron semiconductor detector material. The performance of the detector is affected by the carrier mobility-lifetime product. Therefore, defects that function as carrier recombination center need to be identified. In the presentation, the crystals were grown from melt by the vertical Bridgman method, and characterized by photo-induced current transient spectroscopy (PICTS), low-temperature photoluminescence (LTPL) and detector performance measurement. PICTS measurements revealed electron-related defects located at 0.22, 0.36 and 0.55 eV and hole-related defects at 0.19, 0.30, and 0.73 eV. The defect values are consistent with those measured from LTPL donor-acceptor pair emissions. The carrier mobility-lifetime products were extracted from DC photocurrent and alpha-particle response measurements. This work was partial supported by the Y-12 National Security Complex Plant Directed Research and Development Program No. 630001269, DOE Grant No. 1089091, and the Army Grant No. W911NF-11-0196.

  4. Deviation from Universality in Collisions of Ultracold 6Li2 Molecules

    NASA Astrophysics Data System (ADS)

    Wang, Tout; Heo, Myoung-Sun; Rvachov, Timur; Cotta, Dylan; Ketterle, Wolfgang

    2013-05-01

    Collisions of 6Li2 molecules reveal a striking deviation from universal predictions based on long-range van der Waals interactions. Li2 closed-channel molecules are formed in the highest vibrational state near a narrow Feshbach resonance, and decay via two-body collisions with Li2, Li, and Na. For Li2+Li2 and Li2+Na, the decay rates agree with the universal predictions of the quantum Langevin model. In contrast, the rate for Li2+Li is exceptionally small, with an upper bound ten times smaller than the universal prediction. This can be explained by the low density of available decay states in systems of light atoms [G. Quéméner, J.-M. Launay, and P. Honvault, Phys. Rev. A 75, 050701 (2007)], for which such collisions have not been studied before. Financial support from an AFOSR MURI on Ultracold Molecules, an ARO MURI on Quantum Control of Chemical Reactions, the NSF and the ONR, ARO Grant No. W911NF-07-1-0493, with funds from the DARPA Optical Lattice Emulator program, and NSERC.

  5. High accuracy ab initio studies of Li6+, Li6-, and three isomers of Li6

    NASA Astrophysics Data System (ADS)

    Temelso, Berhane; Sherrill, C. David

    2005-02-01

    The structures and energetics of Li6+, Li6- and three isomers of Li6 are investigated using the coupled-cluster singles, doubles and perturbative triples [CCSD(T)] method with valence and core-valence correlation consistent basis sets of double- to quadruple-ζ quality (cc-pVXZ and cc-pCVXZ, where X =D-Q). These results are compared with qualitatively different predictions by less reliable methods. Our results conclusively show that the D4h isomer is the global minimum structure for Li6. It is energetically favored over the C5v and D3h structures by about 5.1 and 7.1kcalmol-1, respectively, after the inclusion of the zero-point vibrational energy (ZPVE) correction. Our most accurate total atomization energies are 123.2, 117.6, and 115.7kcalmol-1 for the D4h, C5v, and D3h isomers, respectively. Comparison of experimental optical absorption spectra with our computed electronic spectra also indicate that the D4h isomer is indeed the most stable structure. The cation, anion, and some higher spin states are investigated using the less expensive cc-pCVDZ basis set. Adiabatic ionization energies and electron affinities are reported and compared with experimental values. Predictions of molecular properties are found to be sensitive to the basis set used and to the treatment of electron correlation.

  6. {sup {bold 6}}Li(vector)+{sup {bold 12}}C inelastic scattering at 30 and 50 MeV

    SciTech Connect

    Kerr, P.L.; Kemper, K.W.; Green, P.V.; Mohajeri, K.; Myers, E.G.; Schmidt, B.G.; Hnizdo, V.

    1996-09-01

    A complete set of analyzing powers (AP`s), {ital iT}{sub 11}, {ital T}{sub 20}, {ital T}{sub 21}, and {ital T}{sub 22}, for 50 MeV {sup 12}C({sup 6}Li(vector),{sup 6}Li) elastic scattering and inelastic scattering to the {sup 12}C(2{sup +}, 4.44 MeV), {sup 12}C(0{sup +}, 7.65 MeV), and {sup 12}C(3{sup {minus}}, 9.64 MeV) states over the center-of-mass (c.m.) angular range 10{degree}{endash}115{degree} is reported. In addition, cross sections for the excited states 3{sup +}(2.18 MeV), 2{sup +}(4.31 MeV), and 1{sup +}(5.65 MeV) of {sup 6}Li were measured by using the inverse-kinematics reaction {sup 6}Li({sup 12}C,{sup 12}C) at 100 MeV. A combined analysis of the new 50 MeV data and previous 30 MeV data has been carried out using the coupled-channels (CC) code FRESCO. The CC calculations use an optical potential with double-folded (DF) real central, Woods-Saxon imaginary central, and Thomas real spin-orbit (SO) potentials. Calculations include reorientation terms and coupling to the first three excited states of {sup 6}Li and the first two nonzerospin states of {sup 12}C. The {sup 6}Li coupling strengths were fixed by the measured {sup 6}Li excited-state cross sections. The elastic-scattering cross sections and A.P.`s are described well. The need for an explicit SO potential is apparent in the elastic and inelastic-scattering AP`s {ital iT}{sub 11}, more so at 30 MeV than at 50 MeV. The rank-2 AP`s up to 50{degree} c.m. arise mainly from ground-state reorientation effects. The DF potential normalization constant {ital N} approaches unity for the 50 MeV data. At both energies, the {sup 12}C(2{sup +}) cross sections are underestimated at large angles, and the description of the {sup 12}C(3{sup {minus}}) cross sections is poor in detail. The {sup 12}C(3{sup {minus}}) AP`s and the {sup 12}C(2{sup +}) {ital iT}{sub 11} are not reproduced at either energy. {copyright} {ital 1996 The American Physical Society.}

  7. Measurement of fusion excitation function for 7Li+64Ni near the barrier

    NASA Astrophysics Data System (ADS)

    Moin Shaikh, Md.; Roy, Subinit; Rajbanshi, S.; Mukherjee, A.; Pradhan, M. K.; Basu, P.; Pal, S.; Nanal, V.; Shrivastava, A.; Saha, S.; Pillay, R. G.

    2016-05-01

    Total fusion (TF) excitation function has been measured for the system 7Li + 64Ni at the energies near the Coulomb barrier of the system. The evaporation residue (ER) cross sections have been estimated through the online detection of characteristic γ-rays of the ERs. The summed ER cross sections yielding the experimental TF cross section have been compared with the theoretical one dimensional barrier penetration model (1DBPM) prediction. The measured and the model cross sections are very close to each other at above barrier energies. However, an enhancement of the experimental TF cross section with respect to the 1DBPM prediction is observed at below barrier energies. Coupled channels (CC) calculation with inelastic excitations alone could not explain the enhancement. The origin of the enhancement is identified as due to the enhanced population of the αxn channels.

  8. Dynamics of fragment capture for cluster structures of weakly bound 7Li

    NASA Astrophysics Data System (ADS)

    Shrivastava, A.; Navin, A.; Diaz-Torres, A.; Nanal, V.; Ramachandran, K.; Rejmund, M.; Bhattacharyya, S.; Chatterjee, A.; Kailas, S.; Lemasson, A.; Palit, R.; Parkar, V. V.; Pillay, R. G.; Rout, P. C.; Sawant, Y.

    2013-12-01

    Role of cluster structures of 7Li on reaction dynamics have been studied by performing exclusive measurements of prompt-γ rays from residues with scattered particles at energy, E/Vb = 1.6, with 198Pt target. Yields of the residues resulting after capture of t and 4,5,6He, corresponding to different excitation energies of the composite system were estimated. The results were compared with three body classical-dynamical model for breakup fusion, constrained by the measured fusion, α and t capture cross-sections. The cross-section of residues from capture of α and t agreed well with the prediction of the model showing dominance of the two step process - breakup fusion, while those from tightly bound 6He showed massive transfer to be the dominant mechanism.

  9. Probing the location and distribution of paramagnetic centers in alkali metal-loaded zeolites through (7)Li MAS NMR.

    PubMed

    Terskikh, Victor V; Ratcliffe, Christopher I; Ripmeester, John A; Reinhold, Catherine J; Anderson, Paul A; Edwards, Peter P

    2004-09-15

    The nature and surroundings of lithium cations in lithium-exchanged X and A zeolites following loading with the alkali metals Na, K, Rb, and Cs have been studied through (7)Li solid-state NMR spectroscopy. It is demonstrated that the lithium in these zeolites is stable with respect to reduction by the other alkali metals. Even though the lithium cations are not directly involved in chemical interactions with the excess electrons introduced in the doping process, the corresponding (7)Li NMR spectra are extremely sensitive to paramagnetic species that are located inside the zeolite cavities. This sensitivity makes (7)Li NMR a useful probe to study the formation, distribution, and transformation of such species.

  10. Magnetic fluctuations and possible formation of a spin-singlet cluster under pressure in the heavy-fermion spinel LiV2O4 probed by 7Li and 51V NMR

    NASA Astrophysics Data System (ADS)

    Takeda, Hikaru; Kato, Yusuke; Yoshimura, Masahiro; Shimizu, Yasuhiro; Itoh, Masayuki; Niitaka, Seiji; Takagi, Hidenori

    2015-07-01

    7Li and 51V NMR measurements up to 9.8 GPa have been made to elucidate local magnetic properties of a heavy-fermion spinel oxide LiV2O4 which undergoes a metal-insulator transition above ˜7 GPa. The temperature T and pressure P dependences of the 7Li and 51V Knight shifts and the nuclear spin-lattice relaxation rates 1 /T1 show that in the metallic phase, there is a crossover from a high-T region with weak ferromagnetic fluctuations to a low-T one with antiferromagnetic (AFM) fluctuations. The AFM fluctuations are enhanced below 20 K and 1.5 GPa, where a heavy Fermi-liquid state with the modified Korringa relation is formed. The evolution of the magnetic fluctuations is discussed from the aspect of the competition among several magnetic interactions. Above PMI˜6.7 GPa, we find the coexistence of metallic and insulating phases due to the first-order metal-insulator transition. The 7Li and 51V NMR spectra coming from the insulating phase have T -independent small Knight shifts and 7(1 /T1 ) with the thermally activated T dependence, indicating the formation of a spin-singlet cluster. We propose a model of a spin-singlet tetramer as discussed in geometrically frustrated materials.

  11. Studies of nuclear reaction at very low energies. Technical progress report

    SciTech Connect

    Cecil, F.E.

    1992-01-15

    The deuteron radiative capture reactions on {sup 2}H, {sup 6}Li and {sup 10}B have been measured between center of mass energies of 20 and 140 keV. Of note is the observation that the gamma ray-to-charged particle branching ratio for the DD reaction appears independent of energy down to a center of mass energy of 20 keV, consistent with some and contrary to other theoretical models. We have investigated the ratio of the reactions D(d,p)T and D(d,n){sup 3}He down to c.m. energies of 3 keV and the ratio of the reactions 6Li(d,p){sup 7}Li and {sup 6}LI(d,{alpha}){sup 4}He down to a c.m. energy of 19 keV. The DD reaction ratio is independent of energy while the (d,p) branch of the D-{sup 6}Li evinces a significant enhancement at the lowest measured energies. We have continued our investigation of charged particle production from deuterium-metal systems at a modest level of activity. Noteworthy in this investigation is the observation of 3 MeV protons from deuteron beam loaded Ti and LiD targets subjected to extreme thermal disequilibria. Significant facility improvements were realized during the most recent contract period. Specifically the downstream magnetic analysis system proposed to eliminate beam induced contaminants has been installed and thoroughly tested. This improvement should allow the D(a,{gamma}){sup 6}Li reaction to be measured in the coming contract period. A scattering chamber required for the measurement of the {sup 7}Li({sup 3}He,p){sup 9}Be reaction has been designed, fabricated and installed on the accelerator. A CAMAC based charged particle identification system has been assembled also for use in our proposed measurement of the {sup 7}Li({sup 3}He, p){sup 9}Be.

  12. 6Li breakup from 208Pb target at Coulomb barrier energies: doorway to reaction mechanism induced by loosely bound/halo nuclei

    NASA Astrophysics Data System (ADS)

    Mazzocco, M.; Scopel, P.; Signorini, C.; Fortunato, L.; Soramel, F.; Thompson, I. J.; Vitturi, A.; Barbui, M.; Brondi, A.; Cinausero, M.; Fabris, D.; Fioretto, E.; La Rana, G.; Lunardon, M.; Moro, R.; Ordine, A.; Prete, G. F.; Rizzi, V.; Stroe, L.; Trotta, M.; Vardaci, E.; Viesti, G.

    2004-12-01

    The breakup cross section of the system 6Li + 208Pb has been measured at four beam energies close to the Coulomb barrier and the excitation energy distributions of the α + d/ 6Li * system have been deduced. Comparison of the experimental data with two different theoretical approaches strongly supports the direct breakup process description.

  13. Quasi-monoenergetic neutron energy spectra for 246 and 389 MeV 7Li(p,n) reactions at angles from 0° to 30°

    NASA Astrophysics Data System (ADS)

    Iwamoto, Yosuke; Hagiwara, Masayuki; Satoh, Daiki; Iwase, Hiroshi; Yashima, Hiroshi; Itoga, Toshiro; Sato, Tatsuhiko; Nakane, Yoshihiro; Nakashima, Hiroshi; Sakamoto, Yukio; Matsumoto, Tetsuro; Masuda, Akihiko; Nishiyama, Jun; Tamii, Atsushi; Hatanaka, Kichiji; Theis, C.; Feldbaumer, E.; Jaegerhofer, L.; Pioch, C.; Mares, V.; Nakamura, Takashi

    2011-02-01

    The authors measured the neutron energy spectra of a quasi-monoenergetic 7Li(p,n) neutron source with 246 and 389 MeV protons set at seven angles (0°, 2.5°, 5°, 10°, 15°, 20° and 30°), using a time-of-flight (TOF) method employing organic scintillators NE213 at the Research Center for Nuclear Physics (RCNP) of Osaka University. The energy spectra of the source neutrons were precisely deduced down to 2 MeV at 0° and 10 MeV at other angles. The cross-sections of the peak neutron production reaction at 0° were on the 35-40 mb line of other experimental data, and the peak neutron angular distribution agreed well with the Taddeucci formula. Neutron energy spectra below 100 MeV at all angles were comparable, but the shapes of the continuum above 150 MeV changed considerably with the angle. In order to consider the correction required to derive the response in the peak region from the measured total response for high-energy neutron monitors such as DARWIN and Wendi-2, the authors showed the subtractions of H*(10) obtained at larger angles (10°, 15°, 20° and 30°) from the 0° data in the continuum part for the 246 and 389 MeV 7Li(p,n) reactions. It was found that subtracting the dose equivalent at about 20° from the 0° data almost eliminates the continuum component. This method has potential to eliminate problems associated with continuum correction for high-energy neutron monitors.

  14. Folding model analysis of pion elastic and inelastic scattering from {sup 6}Li and {sup 12}C

    SciTech Connect

    Ebrahim, A. A.

    2013-04-15

    {pi}{sup {+-}}-Nucleus scattering cross sections are calculated applying the Watanabe superposition model with a phenomenological Woods-Saxon potential. The phenomenological potential parameters are searched for {pi}{sup {+-}} scattering from {sup 6}Li and {sup 12}C to reproduce not only differential elastic cross sections but also inelastic and total and reaction cross sections at pion kinetic energies from 50 to 672 MeV. The optical potentials of {sup 6}Li and {sup 12}C are calculated in terms of the alpha particle and deuteron optical potentials. Inelastic scattering has been analyzed using the distorted waves from elastic-scattering data. The values of deformation lengths thus obtained compare very well with the ones reported earlier.

  15. Dynamic polarization potential effects on vector analyzing powers of 6Li- 28Si elastic scattering from non-monotonic potentials

    NASA Astrophysics Data System (ADS)

    Basak, A. K.; Roy, P. K.; Hossain, S.; Abdullah, M. N. A.; Tariq, A. S. B.; Uddin, M. A.; Reichstein, I.; Malik, F. B.

    2010-08-01

    Experimental cross section (CS) and vector analyzing power (VAP) data of the 6Li-28Si elastic scattering at 22.8 MeV are analyzed in the coupled-channels (CC) and coupled discretized continuum channels (CDCC) methods. Non-monotonic (NM) 6Li and α potentials of microscopic origin are employed, respectively, in the CC calculations and to generate folding potentials for the CDCC calculations. The study demonstrates that the use of central NM potentials can generate an appropriate dynamic polarization potential (DPP) required to describe both the CS and VAP data without the necessity of renormalization. This also produces an effective spin-orbit (SO) potential to account for the iT11 data without the requirement of an additional static SO potential at the incident energy considered.

  16. Trojan horse method applied to {sup 9}Be(p,{alpha}){sup 6}Li at astrophysical energies

    SciTech Connect

    Wen Qungang; Li Chengbo; Zhou Shuhua; Meng Qiuying; Zhou Jing; Li Xiaomei; Hu Shouyang; Fu Yuanyong; Spitaleri, C.; Tumino, A.; Pizzone, R. G.; Rapisarda, G. G.

    2008-09-15

    The low-energy bare-nucleus cross section for {sup 9}Be(p,{alpha}){sup 6}Li has been extracted by means of the Trojan horse method (THM) applied to the {sup 2}H({sup 9}Be, {alpha},{sup 6}Li)n reaction at a beam energy of {sup 9}Be of 22.35 MeV. For the first time, we assume an intermediate process, {sup 9}Be+{sup 2}H{yields}{sup 9}Be+p+n, and considered this process as one criterion of the quasifree condition. Accordingly, sequential decay processes were eliminated. The derived astrophysical S(E) factor for the two-body process {sup 9}Be(p,{alpha}){sup 6}Li is compared with that obtained from direct experiments. We have found good agreement between the two results, leading to an improved determination of the S(E) with S(0)=21.0{+-}0.8 MeV b. Furthermore, the electron screening potential energy U{sub e}=676{+-}86 eV has also been extracted in a model-independent way by comparing the direct and THM data. The value is significantly higher than that predicted by current theoretical models, whereas it is lower than Ue{approx_equal}830 eV, which was extracted from direct measurements with inclusion of the E{sub c.m.}=-23 keV subthreshold resonance.

  17. Measurement of the ^7Li(d,n)^8Be Reaction at Astrophysically Relevant Energies

    NASA Astrophysics Data System (ADS)

    Sabourov, A.; Ahmed, M.; Crowell, A.; Howell, C.; Joshi, K.; Nelson, S.; Perdue, B.; Sabourov, K.; Tonchev, A.; Weller, H. R.; Prior, R.; Spraker, M.; Kalantar, N.

    2003-10-01

    We have measured the differential cross section and the polarization observables T_20(θ), T_21(θ), T_22(θ), and iT_11(θ) for the ^7Li(d,n)^8Be reaction at low energies. Polarized deuterons of Ed = 160 keV to 80 keV were stopped in an evaporated lithium target. Nine liquid scintillation detectors were used to detect the emitted neutrons. The present experimental results are being compared to theoretical calculations performed with the DWUCK4 (P.D. Kunz, http://spot.colorado.edu/ ˜kunz/DWBA.html) code. Due to the very low energies of the present experiment, only s- and p-waves are likely to contribute in the entrance channel, limiting the number of transition matrix elements (TMEs) contributing to the reaction. Detailed information on the amplitudes and phases of these TMEs will be obtained by performing a simultaneous fit to the cross section and polarization observables. These results should provide new insight into the dynamics of this reaction at low energies.

  18. Comparison of corrosion behavior of EUROFER and CLAM steels in flowing Pb-15.7Li

    NASA Astrophysics Data System (ADS)

    Konys, J.; Krauss, W.; Zhu, Z.; Huang, Q.

    2014-12-01

    Ferritic martensitic steels are envisaged to be applied as structural materials in HCLL blanket systems. Their compatibility with the liquid breeder, which is in direct contact with the structural alloy, will be essential for reliable and safe operation of the designed blankets. Formerly performed corrosion tests of RAFM steels in PICOLO loop of KIT were mainly done at high flow velocities, e.g., 0.22 m/s and delivered severe attack with material loss rates above 400 μm/yr at 823 K. Meanwhile, flow velocities for corrosion testing have been reduced into the "cm range" to be near fusion relevant conditions. Among the international ITER-partners, many varieties of RAFM steels have been developed and manufactured within the last decade, e.g., the so-called Chinese Low Activation Martensitic steel (CLAM). In this paper, the long term corrosion behavior of EUROFER and CLAM steel in flowing Pb-15.7Li will be presented at a flow velocity of about 0.10 m/s and compared with earlier obtained results of RAFM steels exposed at other operation parameters of PICOLO loop. The observed corrosion attack is near 220 μm/yr and fits well to predictions made by MATLIM-modeling for low flow velocities in the turbulent flow regime.

  19. Mechanisms of the sup 64 Zn(d, sup 6 Li) sup 60 Ni reaction at E sub lab = 16. 4 MeV

    SciTech Connect

    Bowsher, J.E.

    1989-01-01

    Cross-sections, A{sub y}, A{sub yy}, and A{sub xx} for the {sup 64}Zn(d, {sup 6}Li) reaction forming the ground and first excited states of {sup 60}Ni were measured in 5{degree} steps from {theta}{sub lab} = 25{degree} to 80{degree} using an E{sub lab} = 16.4 MeV beam of vector and tensor polarized deuterons. These data include the first measurement of A{sub xx} and A{sub yy} for the (d, {sup 6}Li) reaction on a medium to heavy target nucleus. The A{sub y} measurement is also among the first for (d,{sup 6}Li) reactions. Also measured were excitation functions of d{sigma}/d{Omega}, A{sub y}, A{sub yy}, and A{sub xx} for {sup 64}Zn(d,d) scattering at E{sub lab} = 16.4 MeV. The {sup 6}Li ground state and seven other wave functions, each representing {sup 6}Li continuum states of a given spin, I, and internal orbital angular momentum, l, l {le} 2, were included in coupled-channels (CC) calculations of {sup 60}Ni({sup 6}Li, {sup 6}Li) elastic scattering and finite-range, coupled channel Born approximation (CCBA) calculations for the {sup 64}Zn(d,{sup 6}Li) reaction forming the {sup 60}Ni ground state. This analysis is the first to consider the influence of {sup 6}Li continuum states on the (d, {sup 6}Li) reaction. The {sup 6}Li-{sup 60}Ni interactions were generated using a cluster folding model. Both the folding model and the CC and CCBA calculations were performed by the code FRESCO. For the {sup 64}Zn(d, {sup 6}Li) reaction, CCBA calculations demonstrated that {alpha} transfers forming the 3{sup +} state of {sup 6}Li affect d{sigma}/d{Omega} and A{sub y} very strongly.

  20. Elastic scattering, inelastic excitation, and neutron transfer for 7Li+120Sn at energies around the Coulomb barrier

    NASA Astrophysics Data System (ADS)

    Zagatto, V. A. B.; Lubian, J.; Gasques, L. R.; Alvarez, M. A. G.; Chamon, L. C.; Oliveira, J. R. B.; Alcántara-Núñez, J. A.; Medina, N. H.; Scarduelli, V.; Freitas, A.; Padron, I.; Rossi, E. S.; Shorto, J. M. B.

    2017-06-01

    Experimental angular distributions for the 7Li+120Sn elastic and inelastic (projectile and target excitations) scattering, and for the neutron stripping reaction, have been obtained at ELAB= 20 , 22, 24, and 26 MeV, covering an energy range around the Coulomb barrier (VB(LAB )≈21.4 MeV). Coupled channel and coupled reaction channel calculations were performed and both describe satisfactorily the experimental data sets. The 1/2- state 7Li inelastic excitation (using a rotational model), as well as the projectile coupling to the continuum (α plus a tritium particle) play a fundamental role on the proper description of elastic, inelastic, and transfer channels. Couplings to the one-neutron stripping channel do not significantly affect the theoretical elastic scattering angular distributions. The spectroscopic amplitudes of the transfer channel were obtained through a shell model calculation. The theoretical angular distributions for the one-neutron stripping reaction agreed with the experimental data.

  1. The 7Li(d, p)8Li reaction in inverse kinematics at 5.44 MeV/u

    NASA Astrophysics Data System (ADS)

    Pakou, A.; Keeley, N.; Cappuzzello, F.; Acosta, L.; Agodi, C.; Aslanoglou, X.; Calabrese, S.; Carbone, D.; Cavallaro, M.; Foti, A.; Marquínez-Durán, G.; Martel, I.; Mazzocco, M.; Parascandolo, C.; Pierroutsakou, D.; Rusek, K.; Sgouros, O.; Soukeras, V.; Strano, E.; Zagatto, V. A. B.

    2017-08-01

    New data are presented for the 7Li(d, p)8Li stripping reaction which, together with previously reported elastic scattering data taken in the same experiment, provide a coherent set. These data, plus existing measurements of the elastic scattering and stripping at 6MeV/u were analysed within the same coupled reaction channels scheme. Good descriptions of the stripping data to the 0.0MeV 2^+ and 0.98MeV 1^+ states of 8Li were obtained using a set of < ^8Li| ^7Li + n〉 overlaps taken from the literature, provided that the elastic scattering was also well described. Multi-step reaction paths made significant contributions to the description of the larger angle data. The asymptotic normalisation coefficients are compared with previous determinations.

  2. Optimization parameters for BDE in BNCT using near threshold 7Li(p,n)7Be direct neutrons.

    PubMed

    Bengua, Gerard; Kobayashi, Tooru; Tanaka, Kenichi; Nakagawa, Yoshinobu

    2004-11-01

    The dose contribution of (10)B(n,alpha)(7)Li reaction in BNCT using near threshold (7)Li(p,n)(7)Be direct neutrons can be increased through the use of materials referred to as boron-dose enhancers (BDE). In this paper, possible BDE optimization criteria were determined from the characteristics of candidate BDE materials namely (C(2)H(4))(n), (C(2)H(3)F)(n), (C(2)H(2)F(2))(n), (C(2)HF(3))(n), (C(2)D(4))(n), (C(2)F(4))(n), beryllium metal, graphite, D(2)O and (7)LiF. The treatable protocol depth (TPD) was used as the assessment index for evaluating the effect of these materials on the dose distribution in a medium undergoing BNCT using near threshold (7)Li(p,n)(7)Be direct neutrons. The maximum TPD (TPD(max)) did not exhibit an explicit dependence on material type as evidenced by its small range and arbitrary variations. The dependence of TPD on BDE thickness was influenced by the BDE material used as indicated by the sharply peaked TPD versus BDE thickness curves for materials with hydrogen compared to the broader curves obtained for those without hydrogen. The BDE thickness required to achieve TPD(max) (BDE(TPD(max))) were also found to be thinner for materials with hydrogen. The TPD(max), the dependence of TPD on BDE thickness, and the BDE(TPD(max)) were established as appropriate BDE optimization parameters. Based on these criteria and other practical considerations, the suitable choice as BDE among the candidate materials considered in this study for treatments involving tumors located at shallow depths would be (C(2)H(4))(n) while beryllium metal was judged as more appropriate for treatment of deep-seated tumors.

  3. Probing the role of Skyrme interactions on the fission dynamics of the 6Li + 238U reaction

    NASA Astrophysics Data System (ADS)

    Sharma, Ishita; Kumar, Raj; Sharma, Manoj K.

    2017-06-01

    The performance of selected five Skyrme forces (out of a set of 240), tested by Dutra et al., is analyzed in view of fusion-fission dynamics. These forces are assumed to perform better for neutron-rich systems, so the choice of the reaction is accordingly made by opting for a neutron-rich target in 6Li + 238U reaction. This reaction is diagnosed further in reference to fusion hindrance within the dynamical approach of the cluster-decay model (DCM). In order to reduce the computational time, three Skyrme forces are figured out with the criteria that these forces cover the barrier characteristics of the remaining two forces as well. The fission cross-sections are successfully addressed at low energies for the 6Li + 238U reaction. However, at relatively higher energies, the excitation functions show theoretical suppression with respect to experimental data, which may be associated with the possible existence of incomplete fusion (ICF). For ICF, we have considered that the 6Li broke into 4He + 2H, as mentioned in the experimental work. The calculations of ICF are carried out for the 4He + 238U reaction with the selected Skyrme forces at E_{c.m.} = 26.20 and 27.51 MeV. These forces address the data nicely for the compound nucleus (CN) as well as ICF processes. Here, the NRAPR force seems to require lesser barrier modification as compared to the other forces, therefore it can be used as an alternate choice for calculating the interaction potential. Additionally, the prediction of cross-sections at lower energies has been done with DCM using the NRAPR force. The ℓ-dependent % barrier modification of the Skyrme forces undertaken is also worked out in reference to fusion hindrance at below barrier energies.

  4. Thermoluminescence of 7LiF in therapeutic high linear energy transfer (LET) charged-particle beams.

    PubMed

    Chu, C L; Hogstrom, K R; Chen, G C; Hilko, R L

    1986-02-01

    The thermoluminescence of the 200 and 260 degrees C peaks of 7LiF has been measured and compared with off-axis dose and depth-dose distributions for three therapeutic high-LET beams: negative pions, helium ions and neon ions. The methods of analysis consisted of both a single-peak analysis and the dual-peak analysis methods of Hogstrom and Irifune and Hoffmann et al. The results indicate that 7LiF, analysed by the dual-peak analysis methods, is potentially useful for extracting total dose, high-LET dose, and beam quality of helium-ion and negative-pion beams. For the higher-LET neon beam, differences in sensitivity between the 200 and 260 degrees C peaks of 7LiF were found to be independent of variations in LET within the beam; consequently, only the single-peak analysis method is applicable in which case the dosemeter at best can only estimate total dose.

  5. Electric-field modulation of the magnetically induced {sup 6}Li-{sup 40}K Feshbach resonance

    SciTech Connect

    Xie Ting; Wang Gaoren; Zhang Wei; Huang Yin; Cong Shulin

    2011-09-15

    The effect of an external electric field on the magnetically induced {sup 6}Li-{sup 40}K Feshbach resonance is investigated theoretically by using the asymptotic bound state model (ABM). An electric field can modify the position and width of the Feshbach resonance to varying extent. However, it hardly changes the background scattering length in the case without open-channel resonance. The width of the s-wave resonance resulting from the p-wave bound state becomes narrow under the action of a strong electric field. The effects of electric field on orbital angular momentum and electronic state of the Feshbach molecule are also discussed.

  6. Elastic scattering of ^4He by ^6Li at E(^4He) = 24, 25, and 26 MeV

    NASA Astrophysics Data System (ADS)

    Bartosz, E. E.; Cathers, P. D.; Kemper, K. W.; Maréchal, F.; Rusek, K.

    1998-11-01

    A previous optical model analysis of the elastic scattering of ^4He by ^6Li at E(^4He) = 18.5 MeV (P. V. Green, K. W. Kemper, P. L. Kerr, K. Mohajeri, E. G. Myers, D. Robson, K. Rusek and I. J. Thompson, Phys. Rev. C 53) 2862 (1996)., as well as a cluster-folded continuum- discretized coupled channels analysis (K. Rusek, P. V. Green, P. L. Kerr, and K. W. Kemper, Phys. Rev. C 56) 1895 (1997)., resulted in a good description of the data set, but the optical model analysis yielded a poor description of the 25 MeV elastic scattering data measured at the same time. New elastic and inelastic scattering angular distribution cross sections are reported for ^4He + ^6Li at E(^4He) = 24, 25 and 26 MeV. Three energies were used to rule out anomalous scattering at 25 MeV. The results of a cluster-folded continuum- discretized coupled channels analysis similar to that used with the 18.5 MeV data are presented for the three new data sets at 24, 25, and 26 MeV.

  7. Collective-coupling analysis of spectra of mass-7 isobars: {sup 7}He, {sup 7}Li, {sup 7}Be, and {sup 7}B

    SciTech Connect

    Canton, L.; Pisent, G.; Amos, K.; Karataglidis, S.; Svenne, J. P.; Knijff, D. van der

    2006-12-15

    A nucleon-nucleus interaction model has been applied to ascertain the underlying character of the negative-parity spectra of four isobars of mass-7, from neutron- to proton-emitter drip lines. With a single nuclear potential defined by a simple coupled-channel model, a multichannel algebraic scattering approach (MCAS) has been used to determine the bound and resonant spectra of the four nuclides, of which {sup 7}He and {sup 7}B are particle unstable. Incorporation of Pauli blocking into the model enables a description of all known spin-parity states of the mass-7 isobars. We have also obtained spectra of similar quality by using a large space no-core shell model. Additionally, we have studied {sup 7}Li and {sup 7}Be using a dicluster model. We have found a dicluster-model potential that can reproduce the lowest four states of the two nuclei, as well as the relevant low-energy elastic scattering cross sections. But, with this model, the rest of the energy spectra cannot be obtained.

  8. 7Li and 14N NMR studies of phase II-III transition in LiNH4SO4 single crystals

    NASA Astrophysics Data System (ADS)

    Lim, Ae Ran

    2016-12-01

    The NMR spectra of 7Li and 14N nuclei in LiNH4SO4 crystals were obtained near the phase transition temperature TC2=284.5 K. Below TC2, the two physically inequivalent Li groups in phase III were distinguished in 7Li NMR spectra. Meanwhile, the 14N NMR spectra in phase II above TC2 showed four pairs of lines, where as those in phase III showed eight pairs. These changes in the resonance frequencies near TC2 were attributed to the structural phase transition. The 7Li and 14N nuclei in the structure are coordinated through the Li-O-H-N skeleton. Therefore, changes in their NMR spectra with temperature are correlated. The displacements of 7Li and 14N in LiNH4SO4 crystals play important roles in the phase transition near TC2.

  9. Improved information on the 7Li+p{yields}{alpha}+{alpha} reaction via the Trojan Horse Method applied to the 3He break-up

    SciTech Connect

    Tumino, A.; Spitaleri, C.; Sergi, M. L.; Cherubini, S.; La Cognata, M.; Lamia, L.; Pizzone, R. G.; Romano, S.; Tudisco, S.; Kroha, V.; Burjan, V.; Novac, J.; Vincour, J.; Fulop, S.; Somorjai, E.

    2006-04-26

    The astrophysically relevant 7Li+p{yields}{alpha}+{alpha} reaction was investigated via the THM by selecting the quasi-free contribution to the measured 3He+7Li{yields}{alpha}+{alpha}+d three-body process. This investigation is mainly aimed at testing the validity of the pole approximation in the THM against the bound structure of the Trojan-horse nucleus. The three-body experiment was performed at 33 MeV, corresponding to a 7Li-p relative energy ranging from 0.2 to 7 MeV. The quasi-free 7Li+p cross-section was compared with the free reaction cross-section as well as with indirect data from a previous THM experiment. The good agreement between data sets throughout the energy range investigated provided a very important validity test of the pole approximation for the THM.

  10. Irradiation characteristics of BNCT using near-threshold 7Li(p, n)7Be direct neutrons: application to intra-operative BNCT for malignant brain tumours.

    PubMed

    Tanaka, Kenichi; Kobayashi, Tooru; Sakurai, Yoshinori; Nakagawa, Yoshinobu; Ishikawa, Masayori; Hoshi, Masaharu

    2002-08-21

    A calculation method for the dosage of neutrons by near-threshold 7Li(p, n)7Be and gamma rays by 7Li(p, p'gamma)7Li was validated through experiments with variable distance between the Li target and the phantom, focusing on large angular dependence. The production of neutrons and gamma rays in the Li target was calculated by Lee's method and their transport in the phantom was calculated using the MCNP-4B code. The dosage in intra-operative boron neutron capture therapy (BNCT) using near-threshold 7Li(p, n)7Be direct neutrons was evaluated using the validated calculation method. The effectiveness of the usage of the direct neutrons was confirmed from the existence of the region satisfying the requirements of the protocol utilized in intra-operative BNCT for brain tumours in Japan. The boron-dose enhancer (BDE) introduced in this paper to increase the contribution of the 10B(n, alpha)7Li dose in the living body was effective. The void utilized to increase the dose in deep regions was also effective with BDE. For the investigation of 1.900 MeV proton beams, for example, it was found that intraoperative BNCT using near-threshold 7Li(p, n)7Be direct neutrons is feasible.

  11. Absolute frequencies of the {sup 6,7}Li 2S {sup 2}S{sub 1/2}{yields}3S {sup 2}S{sub 1/2} transitions

    SciTech Connect

    Lien, Yu-Hung; Lo, Kuan-Ju; Chen, Jun-Ren; Liu, Yi-Wei; Chen, Hsuan-Chen; Tian, Jyun-Yu; Shy, Jow-Tsong

    2011-10-15

    The measurement of the absolute frequencies of the 2S{yields}3S of atomic lithium is reported. To reduce systematic effects, we employed a frequency-comb-stabilized excitation laser, a weakly collimated atomic beam, and the cascading 2P{yields}2S 670 nm fluorescence as the signal. The transition frequencies, including two isotopes ({sup 6,7}Li), were measured to an accuracy of < 330 kHz. In comparison with the previous GSI Group experiment, the frequency of the 2S{sub 1/2}{yields}3S{sub 1/2} transition of {sup 7}Li is 815 618 181.45(9) MHz, which is improved by a factor of 2. The resultant hyperfine constants of the 3S state and the deduced difference of the nuclear charge radii {delta} from the isotope shift are in good agreement with previous results. Since a more straightforward methodology is adopted, our measurement is less model dependent and serves as an independent investigation of the reported transitions.

  12. Ab initio no-core properties of 7Li and 7Be with the JISP16 and chiral NNLOopt interactions

    NASA Astrophysics Data System (ADS)

    Heng, Taihua; Vary, James P.; Maris, Pieter

    2017-01-01

    We investigate the properties of 7Li with the JISP16 and chiral NNLOopt at next-to-next-to-leading order (NNLO) nucleon-nucleon interactions and 7Be with the JISP16 interaction in the ab initio no-core full configuration approach. We calculate selected observables that include energy spectra, point proton root-mean-square radii, electromagnetic moments, and transitions. We compare our results with experimental results, where available, as well as with results obtained using nucleon-nucleon plus three-nucleon interactions. We obtain reasonable agreement between theory and experiment for low-lying states that are dominated by p -shell configurations.

  13. The Bare Astrophysical S(E) Factor of the 7Li(p, α)α Reaction

    NASA Astrophysics Data System (ADS)

    Lattuada, M.; Pizzone, R. G.; Typel, S.; Figuera, P.; Miljanić, Đ.; Musumarra, A.; Pellegriti, M. G.; Rolfs, C.; Spitaleri, C.; Wolter, H. H.

    2001-12-01

    The astrophysically important 7Li(p, α)α reaction has been studied via the Trojan horse method in the energy range E=10-400 keV. A new theoretical description, based on the distorted-wave Born approximation approach, allows one to extract information on the bare astrophysical S-factor, Sb(E), with Sb(0)=55+/-3 keV barns. The results are compared with direct experimental data leading to a model-independent value of the electron screening potential energy, Ue=330+/-40 eV, much higher than the adiabatic limit Uad=175 eV.

  14. A TPD and AR based comparison of accelerator neutron irradiation fields between (7)Li and W targets for BNCT.

    PubMed

    Tanaka, Kenichi; Endo, Satoru; Yonai, Shunsuke; Baba, Mamoru; Hoshi, Masaharu

    2014-06-01

    The characteristics of moderator assembly dimension was investigated for the usage of (7)Li(p,n) neutrons by 2.3-2.8MeV protons and W(p,n) neutrons by 50MeV protons. The indexes were the treatable protocol depth (TPD) and advantage depth (AD). Consequently, a configuration for W target with the Fe filter, Fluental moderator, Pb reflector showed the TPD of 5.8cm and AD of 9.3cm. Comparable indexes were found for the Li target in a geometry with the MgF2 moderator and Teflon reflector.

  15. Elastic Scattering Of {sup 6,7}Li+{sup 80}Se At Near And Above Barrier Energies

    SciTech Connect

    Fimiani, L.; Marti, G. V.; Capurro, O. A.; Barbara, E. de; Testoni, J. E.; Zalazar, L.; Arazi, A.; Cardona, M. A.; Carnelli, P.; Figueira, J. M.; Hojman, D.; Martinez Heimann, D.; Negri, A. E.; Pacheco, A. J.; Fernandez Niello, J. O.

    2010-08-04

    In this work we propose to study the elastic scattering of the weakly bound projectiles {sup 6,7}Li on an intermediate mass target {sup 80}Se. From the experimental results presented here, precise angular distributions at energies below, around and above the nominal Coulomb barriers of the systems were obtained. The final goal of our work is to determine the characteristic parameters of the optical potential and use them to address the question of whether the usual threshold anomaly or the breakup threshold anomaly are present or not in these systems.

  16. Epithermal neutron beams from the 7 Li(p,n) reaction near the threshold for neutron capture therapy

    NASA Astrophysics Data System (ADS)

    Porras, I.; Praena, J.; Arias de Saavedra, F.; Pedrosa, M.; Esquinas, P.; L. Jiménez-Bonilla, P.

    2016-11-01

    Two applications for neutron capture therapy of epithermal neutron beams calculated from the 7Li ( p , n reaction are discussed. In particular, i) for a proton beam of 1920 keV of a 30 mA, a neutron beam of adequate features for BNCT is found at an angle of 80° from the forward direction; and ii) for a proton beam of 1910 keV, a neutron beam is obtained at the forward direction suitable for performing radiobiology experiments for the determination of the biological weighting factors of the fast dose component in neutron capture therapy.

  17. Quasi-elastic Scattering Measurements in the {sup 6,7}Li+{sup 144}Sm Systems

    SciTech Connect

    Capurro, O. A.; Arazi, A.; Fernandez Niello, J. O.; Figueira, J. M.; Marti, G. V.; Martinez Heimann, D.; Negri, A. E.; Pacheco, A. J.; Monteiro, D. S.; Otomar, D. R.; Gomes, P. R. S.

    2009-06-03

    In the present work, results of measurements of quasi-elastic scattering cross sections using a silicon-telescope detector at backward angles are reported. They allowed us to deduce fusion barrier distributions from the first derivative of the corresponding excitation function (-d(d{sigma}{sub qes}/d{sigma}{sub Rut})/dE). We report data for the systems {sup 6,7}Li on {sup 144}Sm which are characterized by loosely bound projectiles onto a closed neutron shell target. The experimental excitation functions and the associated barrier distributions are compared for both systems.

  18. Breakup threshold anomaly in the near-barrier elastic scattering of {sup 6}Li+{sup 116,112}Sn

    SciTech Connect

    Deshmukh, N. N.; Mukherjee, S.; Patel, D.; Singh, N. L.; Rath, P. K.; Nayak, B. K.; Biswas, D. C.; Santra, S.; Mirgule, E. T.; Danu, L. S.; Gupta, Y. K.; Saxena, A.; Choudhury, R. K.; Kumar, R.; Lubian, J.; Lopes, C. C.; Cardozo, E. N.; Gomes, P. R. S.

    2011-02-15

    We have measured the elastic scattering of the weakly bound {sup 6}Li on the {sup 116,112}Sn targets, at energies close to the Coulomb barrier. The energy dependence of the interaction potential has been investigated by two different methods and the presence of the breakup threshold anomaly is observed. We have also derived the total reaction cross sections for the above systems and compared them to those of other systems with halo, weakly bound, and tightly bound projectiles on targets with similar masses. The reaction cross sections are largest for systems with halo nuclei, then the systems with no-halo weakly bound nuclei, and the smallest cross sections are those for tightly bound systems.

  19. Three-Body Calculation of the 4He(3H,γ)7 Li and 4He(3He,γ)7 Be Reactions and Structure of the 7Li and 7Be at Solar Energies

    NASA Astrophysics Data System (ADS)

    Sadeghi, H.; Khalili, H.

    2014-01-01

    The two 3H+4He and 3He+4He fusion reactions at low energies are usually viewed as an approximate external capture process. We study the 4He(3H,γ)7 Li and 4He(3He,γ)7 Be reactions in a cluster model, which can take into account two- and three-body electromagnetic currents, using minimal substitution in the explicit momentum dependence of the two- and three-cluster interactions. Our main goal is to explore how the cross section of the low-energy 3H+4He or 3He+4He capture reactions depends on energy. The astrophysical S-factors for these reactions are calculated at very low energies. We construct the conserved realistic Argonne v18 for two nucleons and Urbana IX or Tucson-Melbourne three-cluster interactions, which are considered for calculation. We also calculate the binding energies and the structural properties of 3H+4He or 3He+4He systems. The binding energies are found to be -37.72 (-36.32) MeV and -39.35 (-37.43) MeV, with (without) three-body interactions for 7Be and 7Li, in satisfactory agreement with other theoretical results and experimental data, respectively.

  20. Low-energy R -matrix fits for the 6Li(d ,α ) 4HeS factor

    NASA Astrophysics Data System (ADS)

    Grineviciute, J.; Lamia, L.; Mukhamedzhanov, A. M.; Spitaleri, C.; La Cognata, M.

    2015-01-01

    Background: Information about the 6Li(d ,α ) 4He reaction rates of astrophysical interest can be obtained by extrapolating direct data to lower energies, or by indirect methods. The indirect Trojan horse method, as well as various R -matrix and polynomial fits to direct data, estimate electron screening energies much larger than the adiabatic limit. Calculations that include the subthreshold resonance estimate smaller screening energies. Purpose: Obtain the 6Li(d,α ) 4He reaction R -matrix parameters and the bare astrophysical S factor for energies relevant to the stellar plasmas by fitting R -matrix formulas for the subthreshold resonances to the S -factor data above 60 keV. Methods: The bare S factor is calculated using the single- and the two-level R -matrix formulas for the closest to the threshold 0+ and 2+ subthreshold states at 22.2 ,20.2 , and 20.1 MeV. The electron screening potential U e is then obtained by fitting it as a single parameter to the low-energy data. The calculations are also done by fitting U e simultaneously with other parameters. Results: The low-energy S factor is dominated by the 2+ subthreshold resonance at 22.2 MeV. The influence of the other two subthreshold states is small. The resultant electron screening is smaller than the adiabatic value. The fits that neglect the electron screening above 60 keV produce a significantly smaller electron screening potential. The calculations show a large ambiguity associated with a choice of the initial channel radius. Conclusions: The R -matrix fits do not show a significantly larger Ue than predicted by the atomic physics models. The R -matrix best fit provides U e=149.5 eV and Sb(0 ) =21.7 MeV b.

  1. AN UPDATED {sup 6}Li(p, {alpha}){sup 3}He REACTION RATE AT ASTROPHYSICAL ENERGIES WITH THE TROJAN HORSE METHOD

    SciTech Connect

    Lamia, L.; Spitaleri, C.; Sergi, M. L.; Pizzone, R. G.; Tumino, A.; La Cognata, M.; Tognelli, E.; Degl'Innocenti, S.; Prada Moroni, P. G.; Pappalardo, L.

    2013-05-01

    The lithium problem influencing primordial and stellar nucleosynthesis is one of the most interesting unsolved issues in astrophysics. {sup 6}Li is the most fragile of lithium's stable isotopes and is largely destroyed in most stars during the pre-main-sequence (PMS) phase. For these stars, the convective envelope easily reaches, at least at its bottom, the relatively low {sup 6}Li ignition temperature. Thus, gaining an understanding of {sup 6}Li depletion also gives hints about the extent of convective regions. For this reason, charged-particle-induced reactions in lithium have been the subject of several studies. Low-energy extrapolations of these studies provide information about both the zero-energy astrophysical S(E) factor and the electron screening potential, U{sub e} . Thanks to recent direct measurements, new estimates of the {sup 6}Li(p, {alpha}){sup 3}He bare-nucleus S(E) factor and the corresponding U{sub e} value have been obtained by applying the Trojan Horse method to the {sup 2}H({sup 6}Li, {alpha} {sup 3}He)n reaction in quasi-free kinematics. The calculated reaction rate covers the temperature window 0.01 to 2T{sub 9} and its impact on the surface lithium depletion in PMS models with different masses and metallicities has been evaluated in detail by adopting an updated version of the FRANEC evolutionary code.

  2. Calibration of the radiation monitors from DESY and SPring-8 at the quasi-mono-energetic neutron beams using 100 and 300 MeV 7Li(p,n) reaction at RCNP in Osaka Japan in November 2014

    NASA Astrophysics Data System (ADS)

    Leuschner, Albrecht; Asano, Yoshihiro; Klett, Alfred

    2017-09-01

    At the ring cyclotron facility of the Research Center for Nuclear Physics (RCNP) Osaka University, Osaka, Japan a series of measurement campaigns had been continued with quasi mono-energetic neutron beams in November 2014. A 7Li target was bombarded with 100 and 300 MeV protons and the generated neutron beams were directed into a long time-of-flight tunnel at 0 and 25 degrees deflection angle with respect to the proton beam. At a distance of 41 m the cross section of the neutron beam was large enough for the illumination of square meter sized objects like extended range rem-counters. The research institutes SPring-8/RIKEN, Japan, and DESY, Germany, participated in this campaign for the calibration of 4 different types of active ambient dose rate monitors: LB 6411, LB 6411-Pb, LB 6419 and LB 6420. The measurements of their responses are reported and compared with the calculated values.

  3. Two-dimensional diffusion in Li0.7NbS2 as directly probed by frequency-dependent 7Li NMR.

    PubMed

    Epp, V; Nakhal, S; Lerch, M; Wilkening, M

    2013-05-15

    Li ion diffusion in layer-structured Li0.7NbS2 has been complementary investigated by nuclear magnetic resonance (NMR) spectroscopy from an atomic scale point of view. In the present case, (7)Li NMR spin-lattice relaxation (SLR) rates R1ρ probed in the rotating frame of reference proved very informative in characterizing the Li self-diffusion process in the van der Waals gap between the NbS2 layers. While temperature-variable SLRρ measurements were used to determine dynamic parameters such as jump rates (τ(-1)) and the activation energy (Ea), frequency-dependent measurements were used to specify the dimensionality of the diffusion process. In particular, the effect of annealing, i.e., the distribution of Li ions between the layers, on overall Li dynamics has been studied. When plotted in an Arrhenius diagram, the R1ρ rates of an annealed sample, which were recorded at a locking frequency of 20 kHz, pass through a diffusion-induced relaxation peak whose maximum shows up at 320 K. Employing an appropriate diffusion model and appropriately accounting for a non-diffusive background relaxation, a Li jump rate τ(-1)(300 K) ≈ 1.3 × 10(5) s(-1) and an activation energy Ea of 0.43(2) eV can be deduced. Most importantly, in the high-T limit of the diffusion-induced rate peak, i.e., when ω1τ < 1 holds, the rates follow a logarithmic frequency dependence. This points to a diffusion process of low dimensionality and is in good agreement with predictions of relaxation models developed for 2D diffusion.

  4. Atomic frequency comb memory in an isotopically pure 143Nd3+:Y7LiF4 crystal

    NASA Astrophysics Data System (ADS)

    Akhmedzhanov, R. A.; Gushchin, L. A.; Kalachev, A. A.; Korableva, S. L.; Sobgayda, D. A.; Zelensky, I. V.

    2016-01-01

    We implemented the atomic frequency comb protocol for optical quantum memory in an isotopically pure crystal of Y7LiF4 doped by 143Nd3+ ions. Echo signals were observed on the 4I9/2(1)-4F3/2(1) transition, which had inhomogeneous broadening much smaller than the hyperfine splitting of the ground and excited states. We performed hole-burning spectroscopy measurements on several transitions, obtaining information about the hyperfine state lifetimes. An intrinsic hole structure was found on some of the transitions, which allowed us to prepare a comb structure with two clearly defined periods and to observe echo pulses with different time delays.

  5. A tool for calculation of 7Li(p,n)7Be neutron source spectra below the three-body break-up reaction threshold

    NASA Astrophysics Data System (ADS)

    Pachuau, Rebecca; Lalremruata, B.; Otuka, N.; Hlondo, L. R.; Punte, L. R. M.; Thanga, H. H.

    2017-09-01

    We developed a new deterministic neutron source spectrum code EPEN - Energy of Proton Energy of Neutron - for a given lithium target thickness, sample angular coverage and proton energy from the reaction threshold to the three-body break-up threshold. The angular differential cross sections of the 7Li(p,n0)7Be and 7Li(p,n1)7Be reactions evaluated by Liskien and Paulsen were adopted above 1.95 MeV while the functional form suggested by Macklin and Gibbons was adopted for the 7Li(p,n0)7Be reaction cross section near threshold. The spectra obtained by EPEN are validated by the experimental spectra and also compared with the spectra predicted by two Monte Carlo codes, SimLiT and PINO. The results of comparison are discussed in detail.

  6. Measuring the ratio of aqueous diffusion coefficients between [sup 6]Li[sup +]Cl[sup [minus

    SciTech Connect

    Fritz, S.J. )

    1992-10-01

    Osmotic equilibrium is a singular occurrence in the evolution of an osmotic cell because at this event the net solution flux is zero such that [minus]J[sub w] [center dot] [bar V][sub w] = J[sub s] [center dot] [bar V][sub s]. At this juncture, the diffusion coefficient of the solute through the membrane ([omega]) equals the solute flux (J[sub s]) divided by the osmotic pressure ([delta]II). Because the solute permeability coefficient ([omega]) is related to the Fickian diffusion coefficient (D) through the gas constant, temperature, and the membrane's thickness and tortuosity, the ratio of [omega] values for individual isotopic species equals the ratio of D values for the same isotopic components. A 0.9450 molal LiCl solution was placed within sealed dialysis tubing and osmoted against a kilogram of deionized water at 22C. Osmotic equilibrium occurred at 164 [plus minus] 10 min. The ratio of [omega][sub [sup 6]Li[sup +]Cl[sup [minus

  7. Improved neutron-gamma discrimination for a 6Li-glass neutron detector using digital signal analysis methods

    DOE PAGES

    Wang, Cai -Lin; Riedel, Richard A.

    2016-01-14

    A 6Li-glass scintillator (GS20) based neutron Anger camera was developed for time-of-flight single-crystal diffraction instruments at SNS. Traditional pulse-height analysis (PHA) for neutron-gamma discrimination (NGD) resulted in the neutron-gamma efficiency ratio (defined as NGD ratio) on the order of 104. The NGD ratios of Anger cameras need to be improved for broader applications including neutron reflectometers. For this purpose, five digital signal analysis methods of individual waveforms from PMTs were proposed using: i). pulse-amplitude histogram; ii). power spectrum analysis combined with the maximum pulse amplitude; iii). two event parameters (a1, b0) obtained from Wiener filter; iv). an effective amplitude (m)more » obtained from an adaptive least-mean-square (LMS) filter; and v). a cross-correlation (CC) coefficient between an individual waveform and a reference. The NGD ratios can be 1-102 times those from traditional PHA method. A brighter scintillator GS2 has better NGD ratio than GS20, but lower neutron detection efficiency. The ultimate NGD ratio is related to the ambient, high-energy background events. Moreover, our results indicate the NGD capability of neutron Anger cameras can be improved using digital signal analysis methods and brighter neutron scintillators.« less

  8. Improved neutron-gamma discrimination for a {sup 6}Li-glass neutron detector using digital signal analysis methods

    SciTech Connect

    Wang, C. L. Riedel, R. A.

    2016-01-15

    A {sup 6}Li-glass scintillator (GS20) based neutron Anger camera was developed for time-of-flight single-crystal diffraction instruments at Spallation Neutron Source. Traditional Pulse-Height Analysis (PHA) for Neutron-Gamma Discrimination (NGD) resulted in the neutron-gamma efficiency ratio (defined as NGD ratio) on the order of 10{sup 4}. The NGD ratios of Anger cameras need to be improved for broader applications including neutron reflectometers. For this purpose, six digital signal analysis methods of individual waveforms acquired from photomultiplier tubes were proposed using (i) charge integration, (ii) pulse-amplitude histograms, (iii) power spectrum analysis combined with the maximum pulse-amplitude, (iv) two event parameters (a{sub 1}, b{sub 0}) obtained from a Wiener filter, (v) an effective amplitude (m) obtained from an adaptive least-mean-square filter, and (vi) a cross-correlation coefficient between individual and reference waveforms. The NGD ratios are about 70 times those from the traditional PHA method. Our results indicate the NGD capabilities of neutron Anger cameras based on GS20 scintillators can be significantly improved with digital signal analysis methods.

  9. Improved neutron-gamma discrimination for a 6Li-glass neutron detector using digital signal analysis methods

    NASA Astrophysics Data System (ADS)

    Wang, C. L.; Riedel, R. A.

    2016-01-01

    A 6Li-glass scintillator (GS20) based neutron Anger camera was developed for time-of-flight single-crystal diffraction instruments at Spallation Neutron Source. Traditional Pulse-Height Analysis (PHA) for Neutron-Gamma Discrimination (NGD) resulted in the neutron-gamma efficiency ratio (defined as NGD ratio) on the order of 104. The NGD ratios of Anger cameras need to be improved for broader applications including neutron reflectometers. For this purpose, six digital signal analysis methods of individual waveforms acquired from photomultiplier tubes were proposed using (i) charge integration, (ii) pulse-amplitude histograms, (iii) power spectrum analysis combined with the maximum pulse-amplitude, (iv) two event parameters (a1, b0) obtained from a Wiener filter, (v) an effective amplitude (m) obtained from an adaptive least-mean-square filter, and (vi) a cross-correlation coefficient between individual and reference waveforms. The NGD ratios are about 70 times those from the traditional PHA method. Our results indicate the NGD capabilities of neutron Anger cameras based on GS20 scintillators can be significantly improved with digital signal analysis methods.

  10. Hypernuclear production cross section in the reaction of 6Li + 12C at 2 A GeV

    NASA Astrophysics Data System (ADS)

    Rappold, C.; Saito, T. R.; Bertini, O.; Bianchin, S.; Bozkurt, V.; Kim, E.; Kavatsyuk, M.; Ma, Y.; Maas, F.; Minami, S.; Nakajima, D.; Özel-Tashenov, B.; Yoshida, K.; Achenbach, P.; Ajimura, S.; Aumann, T.; Ayerbe Gayoso, C.; Bhang, H. C.; Caesar, C.; Erturk, S.; Fukuda, T.; Göküzüm, B.; Guliev, E.; Hoffmann, J.; Ickert, G.; Ketenci, Z. S.; Khaneft, D.; Kim, M.; Kim, S.; Koch, K.; Kurz, N.; Le Fèvre, A.; Mizoi, Y.; Nungesser, L.; Ott, W.; Pochodzalla, J.; Sakaguchi, A.; Schmidt, C. J.; Sekimoto, M.; Simon, H.; Takahashi, T.; Tambave, G. J.; Tamura, H.; Trautmann, W.; Voltz, S.; Yoon, C. J.

    2015-07-01

    Hypernuclear production cross sections have been deduced for the first time with induced reaction of heavy ion beam on fixed target and by means of the invariant mass method by the HypHI Collaboration exploiting the reaction of 6Li + 12C at 2 A GeV or √{sNN} = 2.70 GeV. A production cross section of 3.9 ± 1.4 μb for 3ΛH and of 3.1 ± 1.0 μb for 4ΛH respectively in the projectile rapidity region was inferred as well as the total production cross section of the Λ hyperon was measured and found to be equal to 1.7 ± 0.8 mb. A global fit based on a Bayesian approach was performed in order to include and propagate statistical and systematic uncertainties. Production ratios of 3ΛH/4ΛH, 3ΛH/Λ and 4ΛH/Λ were included in the inference procedure. The strangeness population factors S3 and S4 of 3ΛH and 4ΛH respectively were extracted. In addition, the multiplicities of the Λ hyperon, 3ΛH, and 4ΛH together with the rapidity and transversal momentum density distributions of the observed hypernuclei were extracted and reported.

  11. Some features and results of thermal neutron background measurements with the [ZnS(Ag)+6LiF] scintillation detector

    NASA Astrophysics Data System (ADS)

    Kuzminov, V. V.; Alekseenko, V. V.; Barabanov, I. R.; Etezov, R. A.; Gangapshev, A. M.; Gavrilyuk, Yu. M.; Gezhaev, A. M.; Kazalov, V. V.; Khokonov, A. Kh.; Panasenko, S. I.; Ratkevich, S. S.

    2017-01-01

    Features of a thermal neutron test detector with thin scintillator [ZnS(Ag)+6LiF] are described. Background of the detector and its registration efficiency were defined as a result of measurements. The thermal neutron flux at different locations, and for different conditions around the Baksan Neutrino Observatory are reported.

  12. Spectroscopic strengths for /sup 6/Li-induced alpha-particle transfers on /sup 18/O at 72 MeV

    SciTech Connect

    Tanabe, T.; Ogino, K.; Kadota, Y.; Haga, K.; Kitahara, T.; Shiba, T.

    1982-08-01

    The /sup 18/O(/sup 6/Li,d)/sup 22/Ne reaction has been studied at 72-MeV bombarding energy. The angular distributions for transitions to low-lying states in /sup 22/Ne are fitted by exact finite-range distorted-wave Born approximation calculations and yield relative spectroscopic factors in good agreement with theoretical predictions.

  13. Novel 4{pi} Detection System for the Measurement of the {sup 6}Li(n,{alpha}){sup 3}H Reaction Cross Section

    SciTech Connect

    Giorginis, Georgios; Bencardino, Raffaele

    2011-12-13

    A dedicated one-dimensional Time Projection Chamber (1D-TPC) was designed and produced at IRMM to determine the {sup 6}Li(n,{alpha}){sup 3}H cross section in the 0.4-2.8 MeV energy range, aiming at 5% accuracy. The basic TPC components were a twin gridded ionisation chamber (GIC) with interwired electrodes and fast digitisation of the anode and cathode signals. The energy of both reaction products emitted from a thin {sup 6}LiF sample at the common TPC cathode was measured. A Kr(97%)CO{sub 2}(3%) mixture was used as the detector gas at a pressure up to 3.5 bar. A {sup 238}U sample mounted on the cathode of an ionisation chamber without grid was used as the neutron flux monitor. Special care was taken to reduce the experimental sources of uncertainty. The beam-monitor {sup 238}U sample was characterised at IRMM by low-geometry {alpha}-counting with an accuracy of 0.1%. A {sup 6}Li sample was produced at IRMM by vacuum evaporation of {sup 6}LiF onto transparent aluminium backing. The number of {sup 6}Li atoms will be measured via Thermal Neutron Depth Profiling with an expected accuracy of 2% with respect to an IRMM Standard Reference Material. First test measurements were performed using a monoenergetic neutron beam produced by the T(p,n){sup 3}He reaction at the IRMM 7 MV Van de Graaff accelerator. The experimental method and preliminary results are presented.

  14. Functions of MgH2 in hydrogen storage reactions of the 6LiBH4-CaH2 reactive hydride composite.

    PubMed

    Zhou, Yifan; Liu, Yongfeng; Zhang, Yu; Gao, Mingxia; Pan, Hongge

    2012-08-28

    A significant improvement of hydrogen storage properties was achieved by introducing MgH(2) into the 6LiBH(4)-CaH(2) system. It was found that ~8.0 wt% of hydrogen could be reversibly stored in a 6LiBH(4)-CaH(2)-3MgH(2) composite below 400 °C and 100 bar of hydrogen pressure with a stepwise reaction, which is superior to the pristine 6LiBH(4)-CaH(2) and LiBH(4) samples. Upon dehydriding, MgH(2) first decomposed to convert to Mg and liberate hydrogen with an on-set temperature of ~290 °C. Subsequently, LiBH(4) reacted with CaH(2) to form CaB(6) and LiH in addition to further hydrogen release. Hydrogen desorption from the 6LiBH(4)-CaH(2)-3MgH(2) composite finished at ~430 °C in non-isothermal model, a 160 °C reduction relative to the 6LiBH(4)-CaH(2) sample. JMA analyses revealed that hydrogen desorption was a diffusion-controlled reaction rather than an interface reaction-controlled process. The newly produced Mg of the first-step dehydrogenation possibly acts as the heterogeneous nucleation center of the resultant products of the second-step dehydrogenation, which diminishes the energy barrier and facilitates nucleation and growth, consequently reducing the operating temperature and improving the kinetics of hydrogen storage.

  15. Isospin transport effects in nuclear reactions at 25 MeV/nucleon

    SciTech Connect

    Lombardo, I.; Cavallaro, S.; Porto, F.; Rizzo, F.; Russotto, P.; Agodi, C.; Alba, R.; Amorini, F.; Anzalone, A.; Di Pietro, A.; Figuera, P.; Han, J.; Maiolino, C.; Santonocito, D.; Berceanu, I.; Pop, A.; Cardella, G.; De Filippo, E.; Pagano, A.; Papa, M.

    2010-07-15

    Isotopic effects are studied in reactions induced by {sup 40}Ca projectiles at 25 MeV/nucleon on {sup 40}Ca, {sup 48}Ca , and {sup 46}Ti targets. The N/Z contents of projectilelike and midvelocity (MV) sources are probed by means of isotopic ({sup 7}Li/{sup 6}Li and {sup 9}Be/{sup 7}Be) and isobaric ({sup 7}Li/{sup 7}Be) yield ratios, for semiperipheral events. In particular, information about isospin transport phenomena will be discussed. Isospin diffusion processes involving nuclei, which have noticeable differences in N/Z have been investigated. Signals of isospin drift, which are related to the gradient of density in the participant region, have also been observed for fragments emitted at MV.

  16. Comparison of the effects of couplings to breakup channels in reactions induced by {sup 6}Li and {sup 6}He on the same {sup 64}Zn target

    SciTech Connect

    Fernández-García, J. P. Di Pietro, A.; Figuera, P.; Fisichella, M.; Lattuada, M.; Musumarra, A.; Pellegriti, M. G.; Scuderi, V.; Torresi, D.; Moro, A. M.; Zadro, M.

    2015-10-15

    The experimental elastic scattering angular distributions for the weakly bound nuclei {sup 6,7}Li and for the halo nucleus {sup 6}He on the same {sup 64}Zn target at several energies around the Coulomb barrier were measured at the Laboratori Nazionali del Sud (LNS, Italy) and at the Cyclotron Research Center, Louvain La Neuve (Belgium), respectively. The measured elastic scattering angular distributions of these three systems at the same center of mass energy have been compared. The experimental data of the {sup 6,7}Li+ {sup 64}Zn systems have been analyzed within the CDCC method, while the {sup 6}He+{sup 64}Zn data have been compared with both both CDCC and CRC calculations.

  17. Nuclear fusion of deuterons with light nuclei driven by Coulomb explosion of nanodroplets

    SciTech Connect

    Ron, Shlomo; Last, Isidore; Jortner, Joshua

    2012-11-15

    Theoretical-computational studies of table-top laser-driven nuclear fusion of high energy (up to 15 MeV) deuterons with {sup 7}Li, {sup 6}Li, T, and D demonstrate the attainment of high fusion yields. The reaction design constitutes a source of Coulomb exploding deuterium nanodroplets driven by an ultraintense, near-infrared, femtosecond Gaussian laser pulse (peak intensity 2 Multiplication-Sign 10{sup 18}-5 Multiplication-Sign 10{sup 19} W cm{sup -2}) and a solid, hollow cylindrical target containing the second reagent. The exploding nanodroplets source is characterized by the deuteron kinetic energies, their number, and the laser energy absorbed by a nanodroplet. These were computed by scaled electron and ion dynamics simulations, which account for intra-nanodroplet laser intensity attenuation and relativistic effects. The fusion yields Y are determined by the number of the source deuterons and by the reaction probability. When laser intensity attenuation is weak within a single nanodroplet and throughout the nanodroplets assembly, Y exhibits a power law increase with increasing the nanodroplet size. Y is maximized for the nanodroplet size and laser intensity corresponding to the 'transition' between the weak and the strong intensity attenuation domains. The dependence of Y on the laser pulse energy W scales as W{sup 2} for weak assembly intensity attenuation, and as W for strong assembly intensity attenuation. This reaction design attains the highest table-top fusion efficiencies (up to 4 Multiplication-Sign 10{sup 9} J{sup -1} per laser pulse) obtained up to date.

  18. (Studies of nuclear reaction at very low energies): Technical progress report

    SciTech Connect

    Cecil, F.E.

    1988-12-14

    We summarize the accomplishments of the first full year's operation of the Colorado School of Mines low energy nuclear physics project utilizing the General Ionex Model 1545 low energy, high current particle accelerator. The projects which we have completed which were explicity included in the original contract proposal include the measurement of the gamma ray branching ratios of the p + /sup 6/Li, p + /sup 7/Li, and p + /sup 11/B reactions as well as the absolute yield of the reaction /sup 9/Be(p,..gamma..)/sup 10/B between proton laboratory energies of about 40 to 180 keV. in the course of these measurements we have demonstrated the associated gamma ray technique for Germanium detector efficiency calibration at gamma ray energies up to 12 MeV using very low energy proton beams. We have, in addition, pursued a fairly comprehensive investigation of an extremely interesting and totally surprising phenomenon in which we see a yield of the d-d fusion reaction during bombardment of deuterated polyethylene by light to medium ion and molecular beams which is greatly enhanced over the yield expected from a straight-forward secondary ion reaction calculation. This enhanced yield is seen to correlate with the beam line pressure, suggesting target heating effects to be the source of the enhancement. In conjunction with a parallel contract with the Applied Plasma Physics Program in the DOE Office of Fusion Energy, we have developed an eight channel fast gamma ray spectrometer utilizing the fluorocarbon liquid scintillator NE226. The system has been operated at total gamma ray count rates up to 2.5 MHz with good energy resolution and with no measured dead-time and acceptable levels of pulse pile-up.

  19. High-power electron beam tests of a liquid-lithium target and characterization study of (7)Li(p,n) near-threshold neutrons for accelerator-based boron neutron capture therapy.

    PubMed

    Halfon, S; Paul, M; Arenshtam, A; Berkovits, D; Cohen, D; Eliyahu, I; Kijel, D; Mardor, I; Silverman, I

    2014-06-01

    A compact Liquid-Lithium Target (LiLiT) was built and tested with a high-power electron gun at Soreq Nuclear Research Center (SNRC). The target is intended to demonstrate liquid-lithium target capabilities to constitute an accelerator-based intense neutron source for Boron Neutron Capture Therapy (BNCT) in hospitals. The lithium target will produce neutrons through the (7)Li(p,n)(7)Be reaction and it will overcome the major problem of removing the thermal power >5kW generated by high-intensity proton beams, necessary for sufficient therapeutic neutron flux. In preliminary experiments liquid lithium was flown through the target loop and generated a stable jet on the concave supporting wall. Electron beam irradiation demonstrated that the liquid-lithium target can dissipate electron power densities of more than 4kW/cm(2) and volumetric power density around 2MW/cm(3) at a lithium flow of ~4m/s, while maintaining stable temperature and vacuum conditions. These power densities correspond to a narrow (σ=~2mm) 1.91MeV, 3mA proton beam. A high-intensity proton beam irradiation (1.91-2.5MeV, 2mA) is being commissioned at the SARAF (Soreq Applied Research Accelerator Facility) superconducting linear accelerator. In order to determine the conditions of LiLiT proton irradiation for BNCT and to tailor the neutron energy spectrum, a characterization of near threshold (~1.91MeV) (7)Li(p,n) neutrons is in progress based on Monte-Carlo (MCNP and Geant4) simulation and on low-intensity experiments with solid LiF targets. In-phantom dosimetry measurements are performed using special designed dosimeters based on CR-39 track detectors.

  20. Vector analyzing power measurement of pion scattering from polarized [sup 7]Li in the region of the [Delta][sub 33] resonance

    SciTech Connect

    Meier, R.; Boschitz, E.; Brinkmoeller, B.; Buehler, J.; Ritt, S.; Wessler, M. ); Konter, J.A.; Mango, S.; van den Brandt, B. ); Efimovykh, V.A.; Kovalev, A.I.; Prokofiev, A.N.; Polyakov, V.V. ); Chaumette, P.; Deregel, J.; Durand, G.; Fabre, J. ); Mach, R. ); Tacik, R. )

    1994-01-01

    The inclusive vector analyzing power [ital iT][sub 11] of [pi][sup +][r arrow][sup 7]Li elastic scattering and inelastic scattering to the 0.47 MeV excited state was measured at several angles for [ital T][sub [pi

  1. Cross-section measurement for the /sup 7/Li(n,n't)/sup 4/He reaction at 14. 74 MeV

    SciTech Connect

    Smith, D.L.; Meadows, J.W.; Bretscher, M.M.; Cox, S.A.

    1984-09-01

    The cross section for the /sup 7/Li(n,n't)/sup 4/He reaction is measured at an average neutron energy of 14.74 MeV, with a resolution of 0.324 MeV, relative to the /sup 238/U neutron-fission cross section. Tritium activities for the irradiated lithium-metal samples (enriched to 99.95% in /sup 7/Li) are deduced using a liquid-scintillation counting method which relies upon the tritiated-water standard from the US National Bureau of Standards. The measured cross section ratio of /sup 7/Li(n,n't)/sup 4/He to /sup 238/U neutron fission is 0.2523 (+- 2.2%). The derived /sup 7/Li(n,n't)/sup 4/He reaction cross section is 0.301 (+- 5.3%) barn, based on the ENDF/B-V value of 1.193 (+- 4.8%) barn for the /sup 238/U neutron-fission cross section. 59 references.

  2. Highly enriched 7Be in the ejecta of Nova Sagittarii 2015 No. 2 (V5668 Sgr) and the Galactic 7Li origin

    NASA Astrophysics Data System (ADS)

    Molaro, P.; Izzo, L.; Mason, E.; Bonifacio, P.; Della Valle, M.

    2016-11-01

    We report on the evidence of highly blueshifted resonance lines of the singly ionized isotope of 7Be II in high resolution UVES spectra of Nova Sagittarii 2015 No. 2 (V5668 Sgr). The resonance doublet lines 7Be II at λλ313.0583, 313.1228 nm are clearly detected in several non-saturated and partially resolved high velocity components during the evolution of the outburst. The total absorption identified with Be II has an equivalent width much larger than all other elements and comparable to hydrogen. We estimate an atomic fraction N(7Be)/N(Ca) ≈ 53-69 from unsaturated and resolved absorption components. The detection of 7Be in several high velocity components shows that 7Be has been freshly created in a thermonuclear runaway via the reaction 3He(α, γ)7Be during the Nova explosion, as postulated by Arnould & Norgaar, however in much larger amounts than predicted by current models. 7Be II decays to 7Li II with a half-life of 53.22 d, comparable to the temporal span covered by the observations. The non-detection of 7Li I requires that 7Li remains ionized throughout our observations. The massive Be II ejecta result into a 7Li production that is ≈ 4.7-4.9 dex above the meteoritic abundance. If such a high production is common even in a small fraction (≈5 per cent) of Novae, they can make all the stellar 7Li of the Milky Way.

  3. Spectrum integrated (n,He) cross section comparisons and least squares analyses for /sup 6/Li and /sup 10/B in benchmark fields

    SciTech Connect

    Schenter, R.E.; Oliver, B.M.; Farrar, H. IV

    1986-06-01

    Spectrum integrated cross sections for /sup 6/Li and /sup 10/B from five benchmark fast reactor neutron fields are compared with calculated values obtained using the ENDF/B-V Cross Section Files. The benchmark fields include the Coupled Fast Reactivity Measurements Facility (CFRMF) at the Idaho National Engineering Laboratory, the 10% Enriched U-235 Critical Assembly (BIG-10) at Los Alamos National Laboratory, the Sigma-Sigma and Fission Cavity fields of the BR-1 reactor at CEN/SCK, and the Intermediate Energy Standard Neutron Field (ISNF) at the National Bureau of Standards. Results from least square analyses using the FERRET computer code to obtain adjusted cross section values and their uncertainties are presented. Input to these calculations include the above five benchmark data sets. These analyses indicate a need for revision in the ENDF/B-V files for the /sup 10/B and /sup 6/Li cross sections for energies above 50 keV.

  4. Defects in {sup 6}LiInSe{sub 2} neutron detector investigated by photo-induced current transient spectroscopy and photoluminescence

    SciTech Connect

    Cui, Yunlong; Bhattacharya, Pijush; Buliga, Vladimir; Tupitsyn, Eugene; Rowe, Emmanuel; Wiggins, Brenden; Johnstone, Daniel; Stowe, Ashley; Burger, Arnold

    2013-08-26

    {sup 6}LiInSe{sub 2} is a promising thermal neutron semiconductor detector material. The performance of the detector is affected by the carrier mobility-lifetime products. Therefore, defects that function as carrier recombination centers need to be identified. In this letter, characterization of defect levels in {sup 6}LiInSe{sub 2} by photo-induced current transient spectroscopy (PICTS) and photoluminescence is reported. PICTS measurements revealed electron-related defects located at 0.22, 0.36, and 0.55 eV and hole-related defects at 0.19, 0.30, and 0.73 eV. Free exciton and donor-acceptor pairs (DAP) emissions were observed. The PICTS defect level values are consistent with those extracted from DAP transitions.

  5. 7Li NMR spectroscopy and ion conduction mechanism in mesoporous silica (SBA-15) composite poly(ethylene oxide) electrolyte

    NASA Astrophysics Data System (ADS)

    Reddy, M. Jaipal; Chu, Peter P.

    A composite of mesoporous silica (SBA-15) with a polyethylene oxide (PEO) polymer electrolyte is examined for use in various electrochemical devices. Incorporation of SBA-15 in a PEO:LiClO 4 polymer electrolyte facilitates salt dissociation, enhances ion conductivity, and improves miscibility between organic and inorganic moieties. Optimized conductivity is found at 10 wt.% SBA-15 composition, above this concentration the conductivity is reduced due to aggregation of a SBA-15:Li rich phase. Heating above melt temperature of PEO allows more of the polymer segments to interact with SBA-15. This results in a greater degree of disorder upon cooling, and the ion conductivity is enhanced. A 7Li MAS NMR study reveals three types of lithium-ion coordination. Two major types of conduction mechanism can be identified: one through conventional amorphous PEO; a second via hopping in a sequential manner by replacing the nearby vacancies ('holes') on the surface (both interior and exterior) of the SBA-15 channels.

  6. Non-Destructive Monitoring of Charge-Discharge Cycles on Lithium Ion Batteries using 7Li Stray-Field Imaging

    PubMed Central

    Tang, Joel A.; Dugar, Sneha; Zhong, Guiming; Dalal, Naresh S.; Zheng, Jim P.; Yang, Yong; Fu, Riqiang

    2013-01-01

    Magnetic resonance imaging provides a noninvasive method for in situ monitoring of electrochemical processes involved in charge/discharge cycling of batteries. Determining how the electrochemical processes become irreversible, ultimately resulting in degraded battery performance, will aid in developing new battery materials and designing better batteries. Here we introduce the use of an alternative in situ diagnostic tool to monitor the electrochemical processes. Utilizing a very large field-gradient in the fringe field of a magnet, stray-field-imaging (STRAFI) technique significantly improves the image resolution. These STRAFI images enable the real time monitoring of the electrodes at a micron level. It is demonstrated by two prototype half-cells, graphite∥Li and LiFePO4∥Li, that the high-resolution 7Li STRAFI profiles allow one to visualize in situ Li-ions transfer between the electrodes during charge/discharge cyclings as well as the formation and changes of irreversible microstructures of the Li components, and particularly reveal a non-uniform Li-ion distribution in the graphite. PMID:24005580

  7. Molecular screening in nuclear reactions

    NASA Astrophysics Data System (ADS)

    Cvetinovic, A.; Lipoglavsek, M.; Markelj, S.; Vesic, J.

    2015-12-01

    The dependence of electron screening in nuclear reactions on projectile or target atomic number has been studied by bombarding different hydrogen-containing targets with beams of 7Li , 11B , and 19F . The largest electron screening potentials were obtained in a graphite target containing hydrogen as an impurity. Some measured potentials are almost two orders of magnitude above the theoretical predictions. To explain the measurements, a new concept of electron screening is introduced.

  8. Measurement and Comparison of the Light Output of Ni-doped 6LiF/ZnS for Use in Neutron Multiplicity Counting

    SciTech Connect

    Behling, Richard S.; Bliss, Mary; Cowles, Christian C.; Kouzes, Richard T.; Lintereur, Azaree; Robinson, Sean M.; Siciliano, Edward R.; Stave, Sean C.; Wang, Zheming

    2016-10-06

    Abstract–Alternatives to 3He for neutron detection have recently become attractive for safeguards applications. Pacific Northwest National Laboratory is developing a neutron multiplicity counter that is based on 6LiF/ZnS. Some of the properties of this material, such as the scintillation light decay time, can be tuned by doping the material with a small amount of nickel. This doping affects other properties of the material, in particular the time dependence of the scintillation light output. To determine whether the nickel-doped or undoped 6LiF/ZnS material would better suit the neutron multiplicity counter system, a series of experiments compared the use of undoped 6LiF/ZnS and a Ni-doped variant using both small samples and full-scale detectors made using the two materials. Both materials were manufactured by Eljen Technology of Sweetwater, Texas. The Ni-doped variant produced less light than the undoped material and had a shorter decay time. For all choices of detection threshold above the electronic noise, the decrease in light output did not affect the detection efficiency of the system.

  9. Ultracold neutron detection with 6Li-doped glass scintillators. NANOSC: A fast ultracold neutron detector for the nEDM experiment at the Paul Scherrer Institute

    NASA Astrophysics Data System (ADS)

    Ban, G.; Bison, G.; Bodek, K.; Chowdhuri, Z.; Geltenbort, P.; Griffith, W. C.; Hélaine, V.; Henneck, R.; Kasprzak, M.; Kermaidic, Y.; Kirch, K.; Komposch, S.; Koss, P. A.; Kozela, A.; Krempel, J.; Lauss, B.; Lefort, T.; Lemière, Y.; Mtchedlishvili, A.; Musgrave, M.; Naviliat-Cuncic, O.; Piegsa, F. M.; Pierre, E.; Pignol, G.; Quéméner, G.; Rawlik, M.; Ries, D.; Rebreyend, D.; Roccia, S.; Rogel, G.; Schmidt-Wellenburg, P.; Severijns, N.; Wursten, E.; Zejma, J.; Zsigmond, G.

    2016-10-01

    This paper summarizes the results from measurements aiming to characterize ultracold neutron detection with 6Li-doped glass scintillators. Single GS10 or GS20 scintillators, with a thickness of 100-200μm, fulfill the ultracold neutron detection requirements with an acceptable neutron-gamma discrimination. This discrimination is clearly improved with a stack of two scintillators: a 6Li-depleted glass bonded to a 6Li-enriched glass. The technique of optical contact bonding is used between the two glasses in order to eliminate the need for optical glue or grease between them. Relative to a 3He Strelkov gas detector, the scintillator's detection efficiency is lower for UCN energies close to the scintillator's Fermi potential (85-100 neV), but becomes larger at higher UCN energies. Coupled to a digital data acquisition system, counting rates up to a few 105 counts/s can be handled. A detector based on such a scintillator stack arrangement was built and has been used in the neutron electric dipole moment experiment at the Paul Scherrer Institute since 2010. Its response for routine runs of the neutron electric dipole moment experiment is presented.

  10. Fast Li ion dynamics in the solid electrolyte Li7 P3 S11 as probed by (6,7) Li NMR spin-lattice relaxation.

    PubMed

    Wohlmuth, Dominik; Epp, Viktor; Wilkening, Martin

    2015-08-24

    The development of safe and long-lasting all-solid-state batteries with high energy density requires a thorough characterization of ion dynamics in solid electrolytes. Commonly, conductivity spectroscopy is used to study ion transport; much less frequently, however, atomic-scale methods such as nuclear magnetic resonance (NMR) are employed. Here, we studied long-range as well as short-range Li ion dynamics in the glass-ceramic Li7 P3 S11 . Li(+) diffusivity was probed by using a combination of different NMR techniques; the results are compared with those obtained from electrical conductivity measurements. Our NMR relaxometry data clearly reveal a very high Li(+) diffusivity, which is reflected in a so-called diffusion-induced (6) Li NMR spin-lattice relaxation peak showing up at temperatures as low as 313 K. At this temperature, the mean residence time between two successful Li jumps is in the order of 3×10(8) s(-1) , which corresponds to a Li(+) ion conductivity in the order of 10(-4) to 10(-3) S cm(-1) . Such a value is in perfect agreement with expectations for the crystalline but metastable glass ceramic Li7 P3 S11 . In contrast to conductivity measurements, NMR analysis reveals a range of activation energies with values ranging from 0.17 to 0.26 eV, characterizing Li diffusivity in the bulk. In our case, through-going Li ion transport, when probed by using macroscopic conductivity spectroscopy, however, seems to be influenced by blocking grain boundaries including, for example, amorphous regions surrounding the Li7 P3 S11 crystallites. As a result of this, long-range ion transport as seen by impedance spectroscopy is governed by an activation energy of approximately 0.38 eV. The findings emphasize how surface and grain boundary effects can drastically affect long-range ionic conduction. If we are to succeed in solid-state battery technology, such effects have to be brought under control by, for example, sophisticated densification or through the preparation

  11. Characteristics of BDE dependent on 10B concentration for accelerator-based BNCT using near-threshold 7Li(p,n)7Be direct neutrons.

    PubMed

    Tanaka, K; Kobayashi, T; Bengua, G; Nakagawa, Y; Endo, S; Hoshi, M

    2004-11-01

    The characteristics boron-dose enhancer (BDE) was evaluated as to the dependence on the (10)B concentration for BNCT using near-threshold (7)Li(p,n)(7)Be direct neutrons. The treatable protocol depth (TPD) was utilized as an evaluation index. MCNP-4B calculations were performed for near-threshold (7)Li(p,n)(7)Be at a proton energy of 1.900MeV and for a polyethylene BDE. Consequently, the TPD was increased by increasing T/N ratio, i.e., the ratio of the (10)B concentration in the tumor ((10)B(Tumor)) to that in the normal tissue ((10)B(Normal)), and by increasing (10)B(Tumor) and (10)B(Normal) for constant T/N ratio. It has been found that the BDE becomes unnecessary from the viewpoint of increasing the TPD, when (10)B(Tumor) is over a certain level.

  12. Optimized therapeutic neutron beam for accelerator-based BNCT by analyzing the neutron angular distribution from (7)Li(p,n)(7)Be reaction.

    PubMed

    Kim, Kyung-O; Kim, Jong Kyung; Kim, Soon Young

    2009-01-01

    Perpendicular neutrons (i.e., solid angle bin of 50-150 degrees ) among ones generated from (7)Li(p,n)(7)Be reaction were used to produce an optimized therapeutic neutron beam for accelerator-based BNCT. A new beam port assembly was also designed to shape the fast neutrons into epithermal ones and to reduce unnecessary radiation including gammas. As a result of a simulation, it is found that a tumor at a depth of 60mm from the head skin could be treated within 5 minutes, if a typical tumor is assumed to be taken about 20RBEGy for therapeutic treatment. It is, thus, expected that the neutrons emitted into the solid angle bin of 50-150 degrees from (7)Li(p,n)(7)Be reaction are very effective in producing epithermal neutron beams for BNCT.

  13. A new measurement of the 7Li(d,p)8Li cross section and consequences for 7Be(p,γ)8B

    NASA Astrophysics Data System (ADS)

    Weissman, L.; Broude, C.; Goldring, G.; Hadar, R.; Hass, M.; Schwamm, F.; Shaanan, M.

    1998-02-01

    A novel scheme for measuring the cross section of the 7Be(p,γ)8B reaction, the major source of high energy neutrinos from the sun, is presented. The scheme involves a strictly uniform particle beam and overcomes some of the recognized experimental uncertainties of previous measurements. A new measurement of σ[7Li(d,p)8Li] has been carried out using this setup, and the present value of σ[7Li(d,p)8Li] = 155(8) mb at the top of the Ed(lab.) = 776 keV resonance is compared with previous measurements. A new issue regarding both the (d,p) and (p,γ) reactions has been examined: reaction-product nuclei which are backscattered out of the target. Measurements and simulations carried out in the course of this investigation are presented and discussed in the context of possible effects on the measured cross sections of these reactions.

  14. Characterization of Hundreds of MeV 7Li(p,n) Quasi-Monoenergetic Neutron Source at RCNP Using a Proton Recoil Telescope and TOF Technique

    NASA Astrophysics Data System (ADS)

    Hagiwara, Masayuki; Iwamoto, Yosuke; Iwase, Hiroshi; Yashima, Hiroshi; Satoh, Daiki; Matsumoto, Tetsuro; Masuda, Akihiko; Nakane, Yoshihiro; Tamii, Atsushi; Shima, Tatsushi; Hatanaka, Kichiji; Nakamura, Takashi

    The peak neutron fluence of a quasi-monoenergetic 7Li(p,n) neutron source at RCNP of Osaka University have been measured for four incident proton energies between 100 and 300 MeV, using a proton recoil telescope (PRT) with event selection by a time-of-flight technique. We deduced the cross section of the peak neutron production reaction, 7Li(p,n0,1)7Be, at 0° and compared with that previously obtained with a time-of-flight (TOF) method employing an organic liquid scintillator. The results obtained with different methods are in agreement within their uncertainties and generally consistent with the other experimental data in several hundreds of MeV region.

  15. Synthesis and optical characterization of LiKB4O7, Li2B6O10, and LiCsB6O10 glasses

    SciTech Connect

    Adamiv, V.; Teslyuk, I.; Dyachok, Ya.; Romanyuk, G.; Krupych, O.; Mys, O.; Martynyuk-Lototska, I.; Burak, Ya.; Vlokh, R.

    2010-10-01

    In the current work we report on the synthesis of LiKB4O7, Li2B6O10, and LiCsB6O10 borate glasses. The results for their piezo-optic, acousto-optic, acoustic, elastic, refractive, optical transmission, and optical resistance properties are also presented. It is shown that some of these glasses represent efficient acousto-optic materials that are transparent down to the vacuum ultraviolet range and highly resistant to laser radiation.

  16. Synthesis and optical characterization of LiKB4O7, Li2B6O10, and LiCsB6O10 glasses.

    PubMed

    Adamiv, V; Teslyuk, I; Dyachok, Ya; Romanyuk, G; Krupych, O; Mys, O; Martynyuk-Lototska, I; Burak, Ya; Vlokh, R

    2010-10-01

    In the current work we report on the synthesis of LiKB(4)O(7), Li(2)B(6)O(10), and LiCsB(6)O(10) borate glasses. The results for their piezo-optic, acousto-optic, acoustic, elastic, refractive, optical transmission, and optical resistance properties are also presented. It is shown that some of these glasses represent efficient acousto-optic materials that are transparent down to the vacuum ultraviolet range and highly resistant to laser radiation.

  17. Au, Bi, Co and Nb cross-section measured by quasimonoenergetic neutrons from p + 7Li reaction in the energy range of 18-36 MeV

    NASA Astrophysics Data System (ADS)

    Majerle, M.; Bém, P.; Novák, J.; Šimečková, E.; Štefánik, M.

    2016-09-01

    Au, Bi, Co and Nb samples were irradiated several times with quasi-monoenergetic neutrons from p + 7Li reaction in the energy range of 18-36 MeV. The activities of the samples were measured with the HPGe detector and the reaction rates were calculated. The cross-sections were extracted using the SAND-II method with the reference cross-sections from the EAF-2010 database. The uncertainties of the final results are discussed.

  18. Indirect determination of Li via 74Ge(n,γ)75mGe activation reaction induced by neutrons from 7Li(p,n)7Be reaction

    NASA Astrophysics Data System (ADS)

    Kumar, Sanjiv; Reddy, G. L. N.; Rao, Pritty; Verma, Rakesh; Ramana, J. V.; Vikramkumar, S.; Raju, V. S.

    2012-03-01

    An indirect method to determine Li by 74Ge(n,γ)75mGe activation reaction induced in a high purity Ge (detector) crystal by neutrons from the 7Li(p,n)7Be reaction in a typical particle-induced γ-ray emission (PIGE) spectroscopy experimental set-up is described. Performed with proton beams of energies in excess of 1.88 MeV, the threshold energy (Eth) of the 7Li(p,n)7Be reaction, the determination involves the activity measurement of 75mGe isotope that has a half-life of 47.7 s and decays with the emission of 139 keV γ-rays. Rapidity, selectivity and sensitivity down to ppm levels are the attractive features of the method. It is a suitable alternative to 7Li(p,p'γ)7Li reaction based PIGE technique in the analyses of matrices that contain light elements such as Be, B, F, Na and Al in significant proportions. Interferences can arise from elements, for example V and Ti, that have Eth ⩽ 1.88 MeV for (p,n) reaction. In the case of elements such as Cu, Mo which have with Eth > 1.88 MeV, the incident proton beam energy can be judiciously selected to avoid or minimize an interference. The method, under optimized irradiation conditions, does not entail a risk of neutron stimulated degradation of the performance of the detector. Besides analytical purposes, the measurement of the 75mGe activity can serve as a powerful tool to monitor even low (˜25 n/cm2 s) thermal neutron fluxes.

  19. {alpha}-cluster states in {sup 38}Ar observed via the {sup 34}S({sup 7}Li,t{alpha}){sup 34}S reaction

    SciTech Connect

    Fukada, M.; Ohmura, M.; Harima, F.; Ogino, K.; Takimoto, K.; Ohkubo, S.

    2005-06-01

    To study the {alpha}-cluster states in the {sup 38}Ar nucleus, angular correlation functions between t and {alpha} in the {sup 34}S({sup 7}Li, t{alpha}){sup 38}Ar reaction have been measured. Seven states at 10.2, 10.8, 11.4, 12.2, 12.7, 14.3, and 15.0 MeV were newly observed.

  20. Evaluation of {sup 235}U, {sup 238}U, {sup 6}Li, and {sup 27}Al Cross Sections

    SciTech Connect

    Chandler, J.R.

    2001-05-17

    Good nuclear data are essential for accurate prediction of reactor parameters. Several cross section libraries are currently available for use with GLASS physics calculations. In recent Mark 15 and Mark 22 studies, cross section data were developed to provide more accurate buckling calculations for Mark 15 and Mark 22 charges. This report documents evaluation of these new data for universal application.

  1. Digital signal processing for a thermal neutron detector using ZnS(Ag):6LiF scintillating layers read out with WLS fibers and SiPMs

    NASA Astrophysics Data System (ADS)

    Mosset, J.-B.; Stoykov, A.; Greuter, U.; Hildebrandt, M.; Schlumpf, N.

    2016-07-01

    We present a digital signal processing system based on a photon counting approach which we developed for a thermal neutron detector consisting of ZnS(Ag):6LiF scintillating layers read out with WLS fibers and SiPMs. Three digital filters have been evaluated: a moving sum, a moving sum after differentiation and a digital CR-RC4 filter. The performances of the detector with these filters are presented. A full analog signal processing using a CR-RC4 filter has been emulated digitally. The detector performance obtained with this analog approach is compared with the one obtained with the best performing digital approach.

  2. Experimental study of the p+{sup 6}Li{yields}{eta}+{sup 7}Be reaction 11.3 MeV above threshold

    SciTech Connect

    Budzanowski, A.; Kliczewski, S.; Siudak, R.; Chatterjee, A.; Jha, V.; Roy, B. J.; Hawranek, P.; Magiera, A.; Jahn, R.; Kilian, K.; Maier, R.; Protic, D.; Ritman, J.; Rossen, P. von; Kirillov, Da.; Machner, H.; Kirillov, Di.; Piskunov, N.; Sitnik, I.; Kolev, D.

    2010-10-15

    The cross section for the reaction p+{sup 6}Li{yields}{eta}+{sup 7}Be was measured at an excess energy of 11.28 MeV above threshold by detecting the recoiling {sup 7}Be nuclei. A dedicated set of focal plane detectors was built for the magnetic spectrograph Big Karl and was used for identification and four-momentum measurement of {sup 7}Be. A differential cross section of nb/(d{sigma}/d{Omega})=[0.69{+-}0.20(stat.){+-}0.20(syst.)] sr for the ground state plus 1/2{sup -} was measured. The result is compared to model calculations.

  3. Role of exchange effects in elastic scattering of. cap alpha. particles and /sup 3/He ions by /sup 6/Li nuclei

    SciTech Connect

    Bragin, V.N.; Burtebaev, N.T.; Dui-brevesebaev, A.D.; Ivanov, G.N.; Sakuta, S.B.; Chuev, V.I.; Chulkov, L.V.

    1986-08-01

    Measurements in the entire angular range are carried out for elastic scattering of ..cap alpha.. particles with energies 36.6 and 50.5 MeV and /sup 3/He ions with energies 34, 50, 60, and 72 MeV by /sup 6/Li nuclei. The experimental data obtained have been analyzed within the framework of the optical model. The contribution to the scattering of the mechanism of elastic transfer of clusters was calculated by the distorted-wave method with a finite interaction radius.

  4. Elastic and inelastic scattering to low-lying states of {sup 58}Ni and {sup 90}Zr using 240-MeV {sup 6}Li

    SciTech Connect

    Krishichayan; Chen, X.; Lui, Y.-W.; Tokimoto, Y.; Button, J.; Youngblood, D. H.

    2010-01-15

    Elastic and inelastic scattering of 240-MeV {sup 6}Li particles from {sup 58}Ni and {sup 90}Zr were measured with the multipole-dipole-multipole spectrometer from 4 deg. <={theta}{sub c.m.}<=43 deg. The elastic scattering data were fitted with the double-folding model using the density-dependent M3Y NN effective interaction and with a phenomenological Woods-Saxon potential. B(E2) and B(E3) values obtained for low-lying 2{sup +} and 3{sup -} states with the double-folding calculations agreed with the adopted values.

  5. Study of polarization in quasi-elastic break-up reaction {sup 6}Li(p,2p){sup 5}He in complete kinematics at 1 GeV

    SciTech Connect

    Prokofiev, A.N.; Aleshin, N.P.; Belostotski, S.L.; Dotsenko, Y.V.; Efimovykh, V.A.; Fedorov, O.Y.; Izotov, A.A.; Kisselev, A.Y.; Komarov, E.N.; Miklukho, O.V.; Murzin, V.I.; Naryshkin, Y.G.; Prokofiev, D.A.; Scheglov, Y.A.; Shvedchikov, A.V.; Zhdanov, A.A.; Zhgun, A.A.

    1995-07-15

    The polarization of recoil protons from the reaction {sup 6}Li(p,2p){sup 5}He at 1 GeV of incident proton beam energy was measured with a new two-arm magnetic spectrometer with a carbon polarimeter. The effective polarization of the P-shell protons of {sup 6}Li nucleus was calculated and found to be in a qualitative agreement with the predictions of the cluster model rather than with those of the shell model.

  6. Experimental analysis of neutron and background gamma-ray energy spectra of 80-400 MeV 7Li(p,n) reactions under the quasi-monoenergetic neutron field at RCNP, Osaka University

    NASA Astrophysics Data System (ADS)

    Iwamoto, Yosuke; Sato, Tatsuhiko; Satoh, Daiki; Hagiwara, Masayuki; Yashima, Hiroshi; Masuda, Akihiko; Matsumoto, Tetsuro; Iwase, Hiroshi; Shima, Tatsushi; Nakamura, Takashi

    2017-09-01

    To develop the 100-400 MeV quasi-monoenergetic neutron field, we measured neutron and unexpected gamma-ray energy spectra of the 7Li(p,n) reaction with 80-389 MeV protons in the 100-m time-of-flight (TOF) tunnel at the Research Center for Nuclear Physics (RCNP) cyclotron facility. Neutron energy spectra with energies above 3 MeV were measured by the TOF method, which had been reported in our previous papers, and photon energy spectra with energies above 0.1 MeV were measured by the automatic unfolding function of the radiation dose monitor DARWIN. For neutron spectra, the contribution of peak intensity to the total intensity integrated with energies above 3 MeV varied between 0.38 and 0.48 in the proton energy range of 80-389 MeV. For gamma-ray spectra, highenergetic gamma-rays at around 70 MeV originated from the decay of π0 were observed with proton energies higher than 200 MeV. For the 246-MeV proton incident reaction, the contribution of gamma-ray dose to neutron dose is negligible because the ratio of gamma-ray dose to neutron dose is 0.014.

  7. Indirect study of the {sup 13}C({alpha},n){sup 16}O reaction via the {sup 13}C({sup 7}Li,t){sup 17}O transfer reaction

    SciTech Connect

    Pellegriti, M. G.; Hammache, F.; Roussel, P.; Audouin, L.; Beaumel, D.; Fortier, S.; Vilmay, M.; Descouvemont, P.; Gaudefroy, L.; Kiener, J.; Lefebvre-Schuhl, A.; Tatischeff, V.; Stanoiu, M.

    2008-04-15

    The {sup 13}C({alpha},n){sup 16}O reaction is considered the main neutron source for the s process in low mass asymptotic giant branch (AGB) stars. In the Gamow peak, the cross section sensitively depends on the 1/2{sup +} subthreshold state of {sup 17}O (E{sub x}=6.356 MeV). In this work, we determined the astrophysical S factor through an evaluation of the {alpha} spectroscopic factor and the corresponding asymptotic normalization factor (ANC) of the 6.356 MeV state using the transfer reaction {sup 13}C({sup 7}Li,t){sup 17}O at two different incident energies. Our result confirms that the contribution of the 1/2{sup +} state is dominant at astrophysical energies. Our reaction rate at T=0.09 GK is slightly lower than the value adopted in the Nuclear Astrophysics Compilation of REaction rates (NACRE), but two times larger than the one obtained in a recent ANC measurement.

  8. Development of a quasi-monoenergetic neutron field using the 7Li(p,n)7Be reaction in the energy range from 250 to 390 MeV at RCNP.

    PubMed

    Taniguchi, S; Nakao, N; Nakamura, T; Yashima, H; Iwamoto, Y; Satoh, D; Nakane, Y; Nakashima, H; Itoga, T; Tamii, A; Hatanaka, K

    2007-01-01

    A quasi-monoenergetic neutron field using the (7)Li(p,n)(7)Be reaction has been developed at the ring cyclotron facility at the Research Center for Nuclear Physics (RCNP), Osaka University. Neutrons were generated from a 10-mm-thick Li target injected by 250, 350 and 392 MeV protons and neutrons produced at 0 degrees were extracted into the time-of-flight (TOF) room of 100-m length through the concrete collimator of 10 x 12 cm aperture and 150 cm thickness. The neutron energy spectra were measured by a 12.7-cm diam x 12.7-cm long NE213 organic liquid scintillator using the TOF method. The peak neutron fluence was 1.94 x 10(10), 1.07 x 10(10) and 1.50 x 10(10) n sr(-1) per muC of 250, 350 and 392 MeV protons, respectively. The neutron spectra generated from various thick (stopping length) targets of carbon, aluminium, iron and lead, bombarded by 250 and 350 MeV protons, were also measured with the TOF method. Although these measurements were performed to obtain thick target neutron yields, they are also used as a continuous energy neutron field. These neutron fields are very useful for characterising neutron detectors, measuring neutron cross sections, testing irradiation effects for various materials and performing neutron shielding experiments.

  9. Natural abundance 17O, 6Li NMR and molecular modeling studies of the solvation structures of lithium bis(fluorosulfonyl)imide/1,2-dimethoxyethane liquid electrolytes

    SciTech Connect

    Wan, Chuan; Hu, Mary Y.; Borodin, Oleg; Qian, Jiangfeng; Qin, Zhaohai; Zhang, Ji-Guang; Hu, Jian Zhi

    2016-03-01

    Natural abundance 17O and 6Li NMR experiments, quantum chemistry and molecular dynamics studies were employed to investigate the solvation structures of Li+ at various concentrations of LiFSI in DME electrolytes in an effort to solve this puzzle. It was found that the chemical shifts of both 17O and 6Li changed with the concentration of LiFSI, indicating the changes of solvation structures with concentration. For the quantum chemistry calculations, the coordinated cluster LiFSI(DME)2 forms at first, and its relative ratio increases with increasing LiFSI concentration to 1 M. Then the solvation structure LiFSI(DME) become the dominant component. As a result, the coordination of forming contact ion pairs between Li+ and FSI- ion increases, but the association between Li+ and DME molecule decreases. Furthermore, at LiFSI concentration of 4 M the solvation structures associated with Li+(FSI-)2(DME), Li+2(FSI-)(DME)4 and (LiFSI)2(DME)3 become the dominant components. For the molecular dynamics simulation, with increasing concentration, the association between DME and Li+ decreases, and the coordinated number of FSI- increases, which is in perfect accord with the DFT results. These results provide more insight on the fundamental mechanism on the very high CE of Li deposition in these electrolytes, especially at high current density conditions.

  10. Natural abundance 17O, 6Li NMR and molecular modeling studies of the solvation structures of lithium bis(fluorosulfonyl)imide/1,2-dimethoxyethane liquid electrolytes

    NASA Astrophysics Data System (ADS)

    Wan, Chuan; Hu, Mary Y.; Borodin, Oleg; Qian, Jiangfeng; Qin, Zhaohai; Zhang, Ji-Guang; Hu, Jian Zhi

    2016-03-01

    Natural abundance 17O and 6Li NMR experiments, quantum chemistry and molecular dynamics studies were employed to investigate the solvation structures of Li+ at various concentrations of LiFSI in DME electrolytes. It was found that the chemical shifts of both 17O and 6Li changed with the concentration of LiFSI, indicating the changes of solvation structures with concentration. For the quantum chemistry calculations, the coordinated cluster LiFSI(DME)2 forms at first, and its relative ratio increases with increasing LiFSI concentration to 1 M. Then the solvation structure LiFSI(DME) become the dominant component. As a result, the coordination of forming contact ion pairs between Li+ and FSI- ion increases, but the association between Li+ and DME molecule decreases. Furthermore, at LiFSI concentration of 4 M the solvation structures associated with Li+(FSI-)2(DME), Li+2(FSI-)(DME)4 and (LiFSI)2(DME)3 become the dominant components. For the molecular dynamics simulation, with increasing concentration, the association between DME and Li+ decreases, and the coordinated number of FSI- increases, which is in perfect accord with the DFT results.

  11. Theoretical analysis of the astrophysical S-factor for the capture reaction α + d → {sup 6}Li + γ in the two-body model

    SciTech Connect

    Tursunov, E. M. Turakulov, S. A.; Descouvemont, P.

    2015-03-15

    Theoretical estimates for the astrophysical S-factor and the rate of the reaction d(α, γ){sup 6}Li were obtained on the basis of the two-body model involving an α−d potential that has a simple Gaussian form and which describes correctly S-, P-, and D-wave phase shifts, the binding energy, and the asymptotic normalization coefficient for the S-wave bound state. The wave functions for the bound and continuum channels were calculated with the aid of the highly precise Numerov algorithm. The results for the contributions of the E1 and E2 transition components reveal a good convergence as the upper limit in the effective integrals increases up to 40 fm. The results obtained for the astrophysical S-factor and the rate of the reaction d(α, γ){sup 6}Li in the temperature range of 10{sup 6}K ≤ T ≤ 10{sup 10} K agree well with the results of the calculations performed by A.M. Mukhamedzhanov and his coauthors [Phys. Rev. C 83, 055805 (2011)] by using the known asymptotic form of the wave function at low energies and a complicated two-body potential at higher energies.

  12. Optimization of the Neutron Detector Design Based on the 6LiF/ZnS(Ag) Scintillation Screens for the GAMMA-400 Space Observatory

    NASA Astrophysics Data System (ADS)

    Gnezdilov, I. I.; Dedenko, G. L.; Ibragimov, R. F.; Idalov, V. A.; Kadilin, V. V.; Kaplun, A. A.; Klemetiev, A. V.; Mukhin, V. I.; Taraskin, A. A.; Turin, E. M.; Zaripov, R. N.

    The Neutron Detector (ND) is a new detector sub-system for the future GAMMA-400 space observatory. It aims to complement the instrument's GAMMA-400 electromagnetic calorimeter (CsI(Tl), total depth is 25.0 X0) in identifying cosmic-ray electrons from ∼ 100 MeV up to 3 TeV. Such electrons are of significant scientific interest, but their identification is complicated by the overwhelmingly more abundant hadronic cosmic rays, hence making significant hadronic rejection power of paramount importance. Particle showers initiated by nuclei in the GAMMA-400 calorimeter have a profile different from an electron-induced electromagnetic cascade, and the hadron rejection power deriving from this difference can be significantly enhanced by making use of the thermal neutron activity at late (>100 ns) times relative to the start of the shower. Indeed hadron-induced showers tend to be accompanied by significantly more neutron activity than electromagnetic showers. In the described ND for capturing thermalized neutrons applied isotope 6Li, which is part of the scintillation screen 6LiF/ZnS(Ag). ND placed are under the electromagnetic calorimeter. The results GEANT4 simulation of the ND shows that ND has high neutron detection efficiency.

  13. Depth absorbed dose and LET distributions of therapeutic {sup 1}H, {sup 4}He, {sup 7}Li, and {sup 12}C beams

    SciTech Connect

    Kempe, Johanna; Gudowska, Irena; Brahme, Anders

    2007-01-15

    The depth absorbed dose and LET (linear energy transfer) distribution of different ions of clinical interest such as {sup 1}H, {sup 4}He, {sup 7}Li, and {sup 12}C ions have been investigated using the Monte Carlo code SHIELD-HIT. The energies of the projectiles correspond to ranges in water and soft tissue of approximately 260 mm. The depth dose distributions of the primary particles and their secondaries have been calculated and separated with regard to their low and high LET components. A LET value below 10 eV/nm can generally be regarded as low LET and sparsely ionizing like electrons and photons. The high LET region may be assumed to start at 20 eV/nm where on average two double-strand breaks can be formed when crossing the periphery of a nucleosome, even though strictly speaking the LET limits are not sharp and ought to vary with the charge and mass of the ion. At the Bragg peak of a monoenergetic high energy proton beam, less than 3% of the total absorbed dose is comprised of high LET components above 20 eV/nm. The high LET contribution to the total absorbed dose in the Bragg peak is significantly larger with increasing ion charge as a natural result of higher stopping power and lower range straggling. The fact that the range straggling and multiple scattering are reduced by half from hydrogen to helium increases the possibility to accurately deposit only the high LET component in the tumor with negligible dose to organs at risk. Therefore, the lateral penumbra is significantly improved and the higher dose gradients of {sup 7}Li and {sup 12}C ions both longitudinally and laterally will be of major advantage in biological optimized radiation therapy. With increasing charge of the ion, the high LET absorbed dose in the beam entrance and the plateau regions where healthy normal tissues are generally located is also increased. The dose distribution of the high LET components in the {sup 7}Li beam is only located around the Bragg peak, characterized by a Gaussian

  14. Breakup coupling effects on near-barrier quasi-elastic scattering of {sup 6,7}Li on {sup 144}Sm

    SciTech Connect

    Otomar, D. R.; Lubian, J.; Gomes, P. R. S.; Monteiro, D. S.; Niello, J. O. Fernandez; Guimaraes, V.; Chamon, L. C.

    2009-09-15

    Excitation functions of quasi-elastic scattering at backward angles have been measured for the {sup 6,7}Li+{sup 144}Sm systems at near-barrier energies, and fusion barrier distributions have been extracted from the first derivatives of the experimental cross sections with respect to the bombarding energies. The data have been analyzed in the framework of continuum discretized coupled-channel calculations, and the results have been obtained in terms of the influence exerted by the inclusion of different reaction channels, with emphasis on the role played by the projectile breakup.

  15. Some nuclear physics aspects of BBN

    NASA Astrophysics Data System (ADS)

    Coc, Alain

    2017-09-01

    Primordial or big bang nucleosynthesis (BBN) is now a parameter free theory whose predictions are in good overall agreement with observations. However, the 7 Li calculated abundance is significantly higher than the one deduced from spectroscopic observations. Nuclear physics solutions to this lithium problem have been investigated by experimental means. Other solutions which were considered involve exotic sources of extra neutrons which inevitably leads to an increase of the deuterium abundance, but this seems now excluded by recent deuterium observations.

  16. Parity-violating α-decay of the 3.56 MeV Jπ, T = 0 +, 1 state of 6Li

    NASA Astrophysics Data System (ADS)

    Csótó, Attila; Langanke, Karlheinz

    1996-02-01

    We study the parity-violating α + d decay of the lowest 0 + state of 6Li in a microscopic three-cluster model. The initial bound and the final scattering states are described consistently within the same model. The parity-violating decay width is calculated in perturbation theory using the parity-nonconserving nucleon-nucleon interaction of Desplanques, Donoghue and Holstein (DDH). We find that the decay width is sensitive to dynamical degrees of freedom which are beyond the α + p + n model, for example, α excitation and breakup. In our full model, which contains breathing excitations of the α particle and 3H+ 3He rearrangement, the parity-nonconserving decay width is Γ αdPNC = 3.97 × 10 -9 eV, using the DDH weak coupling constants.

  17. Study of multipole giant resonances in /sup 90/Zr and /sup 120/Sn in scattering of 93-MeV /sup 6/Li ions

    SciTech Connect

    Venikov, N.I.; Glukhov, Y.A.; Dem'yanova, A.S.; Drozdov, S.I.; Novatskii, V.G.; Ogloblin, A.A.; Sakuta, S.B.; Stepanov, D.N.; Unezhev, V.N.; Yupinov, Y.L.; Brynkush, M.; Grama, K.; Lazer, I.

    1981-04-01

    In the inelastic scattering of /sup 6/Li ions with energy 93 MeV we have investigated the regions of quadrupole and octupole giant isoscalar resonances (E/sub x/approx.63A/sup -1/3/ and E/sub x/approx.30A/sup -13/ MeV, respectively) in the nuclei /sup 90/Zr and /sup 120/Sn. The angular distributions of the resonance groups obtained in the region of angles 12--24/sup 0/ are analyzed by the distorted wave Born approximation. Detailed study of the group at E/sub x/approx.63A/sup -1/3/ favors existence of a monopole giant resonance which is located at an excitation energy approx.76A/sup -1/3/ MeV on the left wing of the quadrupole resonance.

  18. Interference effects between /sup 17/O states populated in the /sup 13/C(/sup 6/Li,d)/sup 17/O*. --> cap alpha. +/sup 13/C reaction

    SciTech Connect

    Cardella, G.; Cunsolo, A.; Foti, A.; Imme, G.; Pappalardo, G.; Raciti, G.; Rizzo, F.; Alamanos, N.; Berthier, B.; Saunier, N.

    1987-12-01

    An analysis of the /sup 13/C(/sup 6/Li,d..cap alpha..)/sup 13/C reaction in the collinear (theta/sub d/ = 0/sup 0/) and noncollinear (theta/sub d/ = 10/sup 0/,8/sup 0/) geometry is made for two peaks observed in the deuteron energy spectrum and corresponding to excitation energies of 16.1 and 13.6 MeV in the /sup 17/O nucleus. It is shown that the reaction proceeds via a direct alpha-transfer process which populates doublets of interfering /sup 17/O levels. Spins, weights, and parities of these levels are obtained by means of a least square procedure.

  19. Elastic and inelastic scattering of 240-MeV {sup 6}Li ions from {sup 40}Ca and {sup 48}Ca and tests of a systematic optical potential

    SciTech Connect

    Krishichayan,; Chen, X.; Lui, Y.-W.; Button, J.; Youngblood, D. H.

    2010-04-15

    Elastic and inelastic scattering of 240-MeV {sup 6}Li particles from {sup 40}Ca and {sup 48}Ca were measured with the multipole-dipole-multipole spectrometer from 4 deg. <=theta{sub c.m.}<=40 deg. Optical potential parameters were obtained by fitting the elastic-scattering data with the double-folding model using the density-dependent M3Y NN effective interaction and B(E2) and B(E3) values obtained for low-lying 2{sup +} and 3{sup -} states agreed with the adopted values. The results are compared with those obtained using potentials derived from the systematics of potentials previously obtained for {sup 24}Mg, {sup 28}Si, {sup 58}Ni, and {sup 90}Zr. Cross sections for excitation of giant resonances were also calculated with the potentials obtained.

  20. Cellular cation transport studied by 6/7Li and 23Na NMR in a porous Mo132 Keplerate type nano-capsule as model system.

    PubMed

    Rehder, Dieter; Haupt, Erhard T K; Müller, Achim

    2008-01-01

    Li+ ions can interplay with other cations intrinsically present in the intra- and extra-cellular space (i.e. Na+, K+, Mg2+ and Ca2+) have therapeutic effects (e.g. in the treatment of bipolar disorder) or toxic effects (at higher doses), likely because Li+ interferes with the intra-/extra-cellular concentration gradients of the mentioned physiologically relevant cations. The cellular transmembrane transport can be modelled by molybdenum-oxide-based Keplerates, i.e. nano-sized porous capsules containing 132 Mo centres, monitored through 6/7Li as well as 23Na NMR spectroscopy. The effects on the transport of Li+ cations through the 'ion channels' of these model cells, caused by variations in water amount, temperature, and by the addition of organic cationic 'plugs' and the shift reagent [Dy(PPP)2](7-) are reported. In the investigated solvent systems, water acts as a transport mediator for Li+. Likewise, the counter-transport (Li+/Na+, Li+/K+, Li+/Cs+ and Li+/Ca2+) has been investigated by 7Li NMR and, in the case of Li+/Na+ exchange, by 23Na NMR, and it has been shown that most (in the case of Na+ and K+, all (Ca2+) or almost none (Cs+) of the Li cations is extruded from the internal sites of the artificial cell to the extra-cellular medium, while Na+, K+ and Ca2+ are partially incorporated.

  1. Lithium ion micrometer diffusion in a garnet-type cubic Li7La3Zr2O12 (LLZO) studied using 7Li NMR spectroscopy

    NASA Astrophysics Data System (ADS)

    Hayamizu, Kikuko; Seki, Shiro; Haishi, Tomoyuki

    2017-01-01

    Mobile lithium ions in a cubic garnet Li7La3Zr2O12 (Al-stabilized) were studied using 7Li NMR spectroscopy for membrane and powder samples, the latter of which was ground from the membrane. Lithium diffusion in a micrometer space was measured using the pulsed-gradient spin-echo 7Li NMR method between 70 and 130 °C. When the observation time (Δ ) was shorter than 20 ms, the echo attenuation showed diffusive diffraction patterns, indicating that the Li+ diffusing space is not free but restricted. For longer Δ, the values of apparent diffusion constant (Dapparent) became gradually smaller to approach an equilibrated value (close to a tracer diffusion constant). In addition, the Dapparent depends on the pulse field gradient strength (g) and became smaller as g became larger. These experimental results suggest that the lithium ions diffuse through Li+ pathways surrounded by stationary anions and lithium ions, and are affected by collisions and diffractions. One-dimensional profiles of the membrane sample of thickness 0.5 mm were observed from 65 to 110 °C and the area intensity, as well as the lithium occurrence near the surface, increased with the increase in temperature. The temperature-dependent area intensity showed a correspondence to the number of Li+ carrier ions estimated from the ionic conductivity and the equilibrated diffusion constant through the Nernst-Einstein relationship.

  2. Evaluation of the /sup 7/Li(n,n't)/sup 4/He cross section for ENDF/B-VI and application to uncertainty analysis

    SciTech Connect

    Young, P.G.; Davidson, J.W.; Muir, D.W.

    1988-01-01

    A new covariance analysis of n+/sup 7/Li cross section data has been completed for Version VI of ENDF/B. The analysis updates our 1981 work for ENDF/B-V.2 to include new data that has become available since that time and to incorporate cross correlations between different experiments. The bulk of the new measured data consists of some 10 new (or newly revised) tritium-production measurements involving about 70 new data points. The new analysis results in only small changes in the previous evaluation of the tritium-production cross section but significantly reduces the magnitudes of uncertainties due to the more extensive and accurate data base that was used. A two-dimensional sensitivity and uncertainty analysis of the Lithium Blanket Module experiments at the LOTUS facility was performed in order to assess the effects of the new /sup 7/Li cross sections on tritium breeding uncertainty in a realistic system. 4 refs., 6 figs., 3 tabs.

  3. Lithium ion micrometer diffusion in a garnet-type cubic Li7La3Zr2O12 (LLZO) studied using (7)Li NMR spectroscopy.

    PubMed

    Hayamizu, Kikuko; Seki, Shiro; Haishi, Tomoyuki

    2017-01-14

    Mobile lithium ions in a cubic garnet Li7La3Zr2O12 (Al-stabilized) were studied using (7)Li NMR spectroscopy for membrane and powder samples, the latter of which was ground from the membrane. Lithium diffusion in a micrometer space was measured using the pulsed-gradient spin-echo (7)Li NMR method between 70 and 130 °C. When the observation time (Δ) was shorter than 20 ms, the echo attenuation showed diffusive diffraction patterns, indicating that the Li(+) diffusing space is not free but restricted. For longer Δ, the values of apparent diffusion constant (Dapparent) became gradually smaller to approach an equilibrated value (close to a tracer diffusion constant). In addition, the Dapparent depends on the pulse field gradient strength (g) and became smaller as g became larger. These experimental results suggest that the lithium ions diffuse through Li(+) pathways surrounded by stationary anions and lithium ions, and are affected by collisions and diffractions. One-dimensional profiles of the membrane sample of thickness 0.5 mm were observed from 65 to 110 °C and the area intensity, as well as the lithium occurrence near the surface, increased with the increase in temperature. The temperature-dependent area intensity showed a correspondence to the number of Li(+) carrier ions estimated from the ionic conductivity and the equilibrated diffusion constant through the Nernst-Einstein relationship.

  4. Determination of astrophysical 7Be(p, γ)8B reaction rates from the 7Li(d, p)8Li reaction

    NASA Astrophysics Data System (ADS)

    Du, XianChao; Guo, Bing; Li, ZhiHong; Pang, DanYang; Li, ErTao; Liu, WeiPing

    2015-06-01

    The 7Be(p, γ)8B reaction plays a central role not only in the evaluation of solar neutrino fluxes but also in the evolution of the first stars. Study of this reaction requires the asymptotic normalization coefficient (ANC) for the virtual decay 8B g.s. → 7Be + p. By using the charge symmetry relation, we obtain this proton ANC with the single neutron ANC of 8Li g.s. →7Li + n, which is determined with the distorted wave Born approximation (DWBA) and adiabatic distorted wave approximation (ADWA) analysis of the 7Li(d, p)8Li angular distribution. The astrophysical S-factors and reaction rates of the direct capture process in the 7Be(p, γ)8B reaction are further deduced at energies of astrophysical relevance. The astrophysical S-factor at zero energy for direct capture, S 17(0), is derived to be (19.9 ± 3.5) eV b in good agreement with the most recent recommended value. The contributions of the 1+ and 3+ resonances to the S-factor and reaction rate are also evaluated. The present result demonstrates that the direct capture dominates the 7Be(p, γ)8B reaction in the whole temperature range. This work provides an independent examination to the current results of the 7Be(p, γ)8B reaction.

  5. Microscopic calculation of the 3He(α,γ)7Be and 3H(α,γ)7Li capture cross sections using realistic interactions.

    PubMed

    Neff, Thomas

    2011-01-28

    The radiative capture cross sections for the 3He(α,γ)7Be and 3H(α,γ)7Li reactions are calculated in the fully microscopic fermionic molecular dynamics approach using a realistic effective interaction that reproduces the nucleon-nucleon scattering data. At large distances bound and scattering states are described by antisymmetrized products of 4He and 3He/3H ground states. At short distances the many-body Hilbert space is extended with additional many-body wave functions needed to represent polarized clusters and shell-model-like configurations. Properties of the bound states are described well, as are the scattering phase shifts. The calculated S factor for the 3He(α,γ)7Be reaction agrees very well with recent experimental data in both absolute normalization and energy dependence. In the case of the 3H(α,γ)7Li reaction the calculated S factor is larger than available experimental data by about 15%.

  6. TPD-based evaluation of near threshold mono-energetic proton energies for the (7)Li(p,n)(7)Be production of neutrons for BNCT.

    PubMed

    Bengua, Gerard; Kobayashi, Tooru; Tanaka, Kenichi; Nakagawa, Yoshinobu; Unesaki, Hironobu

    2006-08-21

    An evaluation of mono-energetic proton energies ranging from 1.885 MeV to 1.920 MeV was carried out to determine the viability of these near threshold energies in producing neutrons for BNCT via the (7)Li(p,n)(7)Be reaction. Neutron fields generated at these proton energies were assessed using the treatable protocol depth (TPD) and the maximum TPD (TPD(max)) as evaluation indices. The heavy charged particle (HCP) dose rate to tumour was likewise applied as a figure of merit in order to account for irradiation time and required proton current. Incident proton energies closer to the reaction threshold generated deeper TPDs compared to higher energy protons when no boron dose enhancers (BDE) were placed in the irradiation field. Introducing a BDE resulted in improved TPDs for high proton energies but their achievable TPD(max) were comparatively lower than that obtained for lower proton energies. In terms of the HCP dose rate to tumour, higher proton energies generated neutron fields that yielded higher dose rates both at TPD(max) and at fixed depths of comparison. This infers that higher currents are required to deliver the prescribed treatment dose to tumours for proton beams with energies closer to the (7)Li(p,n)(7)Be reaction threshold and more achievable proton currents of around 10 mA or less for proton energies from 1.900 MeV and above. The dependence on incident proton energy of the TPD, TPD(max) and the HCP dose rate to tumour with respect to the (10)B concentration in tumour and healthy tissues were also clarified in this study. Increasing the (10)B concentration in tumour while maintaining a constant T/N ratio resulted in deeper TPD(max) where a greater change in TPD(max) was obtained for proton energies closer to the (7)Li(p,n)(7)Be reaction threshold. The HCP dose rates to tumour for all proton energies also went up, with the higher proton energies benefiting more from the increased (10)B concentration.

  7. Evaluation of the characteristics of boron-dose enhancer (BDE) materials for BNCT using near threshold 7Li(p,n)7Be direct neutrons.

    PubMed

    Bengua, Gerard; Kobayashi, Tooru; Tanaka, Kenichi; Nakagawa, Yoshinobu

    2004-03-07

    The characteristics of a number of candidate boron-dose enhancer (BDE) materials for boron neutron capture therapy (BNCT) using near threshold 7Li(p,n)7Be direct neutrons were evaluated based on the treatable protocol depth (TPD), defined in this paper. Simulation calculations were carried out by means of MCNP-4B transport code for candidate BDE materials, namely, (C2H4)n, (C2H3F)n, (C2H2F2)n, (C2HF3)n, (C2D4)n, (C2F4)n, beryllium metal, graphite, D2O and 7LiF. Dose protocols applied were those used for intra-operative BNCT treatment for brain tumour currently used in Japan. The maximum TPD (TPDmax) for each BDE material was found to be between 4 cm and 5 cm in the order of (C2H4)n < (C2H3F)n < (C2H2F2)n < (C2HF3)n < beryllium metal < (C2D4)n < graphite < (C2F4)n < D2O < 7LiF. Based on the small and arbitrary variations in the TPDmax for these materials, an explicit advantage of a candidate BDE material could not be established from the TPDmax alone. The dependence of TPD on BDE thickness was found to be influenced by the type of BDE material. For materials with hydrogen, sharp variations in TPD were observed, while those without hydrogen exhibited more moderate fluctuations in TPD as the BDE thickness was varied. The BDE thickness corresponding to TPDmax (BDE(TPDmax)) was also found to depend on the type of BDE material used. Thicker BDE(TPDmax), obtained mostly for BDE materials without hydrogen, significantly reduced the dose rates within the phantom. The TPDmax, the dependence of TPD on BDE thickness and the BDE (TPDmax) were ascertained as appropriate optimization criteria in choosing suitable BDE materials for BNCT. Among the candidate BDE materials considered in this study. (C2H4)n was judged as the suitable material for near-surface tumours and beryllium metal for deeper tumours based on these optimization criteria and other practical considerations.

  8. Characterization of high-energy quasi-monoenergetic neutron energy spectra and ambient dose equivalents of 80-389 MeV 7Li(p,n) reactions using a time-of-flight method

    NASA Astrophysics Data System (ADS)

    Iwamoto, Yosuke; Hagiwara, Masayuki; Satoh, Daiki; Araki, Shouhei; Yashima, Hiroshi; Sato, Tatsuhiko; Masuda, Akihiko; Matsumoto, Tetsuro; Nakao, Noriaki; Shima, Tatsushi; Kin, Tadahiro; Watanabe, Yukinobu; Iwase, Hiroshi; Nakamura, Takashi

    2015-12-01

    We completed a series of measurements on mono-energetic neutron energy spectra of the 7Li(p,n) reaction with 80-389-MeV protons in the 100-m time-of-flight (TOF) tunnel at the Research Center for Nuclear Physics cyclotron facility. For that purpose, we measured neutron energy spectra of the 80-, 100- and 296-MeV proton incident reactions, which had not been investigated in our previous studies. The neutron peak intensity was 0.9-1.1×1010 neutrons/sr/μC in the incident proton energy region of 80-389 MeV, and it was almost independent of the incident proton energy. The contribution of peak intensity of the spectrum to the total intensity integrated with energies above 3 MeV varied between 0.38 and 0.48 in the incident proton energy range of 80-389 MeV. To consider the correction required to derive a response in the peak region from the measured total responses of neutron monitors in the 100-m TOF tunnel, we proposed the subtraction method using energy spectra between 0° and 25°. The normalizing factor k against 25° neutron fluence to equalize it to 0° neutron fluence in the continuum region ranges from 0.74 to 1.02 depending on the incident proton energy and angle measured. Even without the TOF method, the subtraction method with the k factor almost decreases the response in the continuum region of a neutron spectrum against the total response of neutron monitors.

  9. Identification of Li-Ion Battery SEI Compounds through (7)Li and (13)C Solid-State MAS NMR Spectroscopy and MALDI-TOF Mass Spectrometry.

    PubMed

    Huff, Laura A; Tavassol, Hadi; Esbenshade, Jennifer L; Xing, Wenting; Chiang, Yet-Ming; Gewirth, Andrew A

    2016-01-13

    Solid-state (7)Li and (13)C MAS NMR spectra of cycled graphitic Li-ion anodes demonstrate SEI compound formation upon lithiation that is followed by changes in the SEI upon delithiation. Solid-state (13)C DPMAS NMR shows changes in peaks associated with organic solvent compounds (ethylene carbonate and dimethyl carbonate, EC/DMC) upon electrochemical cycling due to the formation of and subsequent changes in the SEI compounds. Solid-state (13)C NMR spin-lattice (T1) relaxation time measurements of lithiated Li-ion anodes and reference poly(ethylene oxide) (PEO) powders, along with MALDI-TOF mass spectrometry results, indicate that large-molecular-weight polymers are formed in the SEI layers of the discharged anodes. MALDI-TOF MS and NMR spectroscopy results additionally indicate that delithiated anodes exhibit a larger number of SEI products than is found in lithiated anodes.

  10. NMR spin-lattice relaxation study of 7Li and 93Nb nuclei in Ti- or Fe-doped LiNbO3:Mg single crystals

    NASA Astrophysics Data System (ADS)

    Yeom, Tae Ho; Lim, Ae Ran

    2016-04-01

    In this study, to understand the effects of paramagnetic impurities, we investigated the temperature dependent of the spin-lattice relaxation times of pure LiNbO3, LiNbO3:Mg, LiNbO3:Mg/Ti, LiNbO3:Mg/Fe, and LiNbO3:Mg/Fe (thermally treated at 500°C) single crystals. The results for the LiNbO3:Mg single crystals doped with Fe3+ or Ti3+ are discussed with respect to the site distribution and atomic mobility of Li and Nb. In addition, the effects of a thermal treatment on LiNbO3:Mg/Fe single crystals were examined based on the T1 analysis of 7Li and 93Nb. It was found that the presence of impurities in the crystals induced systematic changes of activation energies concerning atomic mobility.

  11. Radiative neutron capture by {sup 2}H, {sup 7}Li, {sup 14}C, and {sup 14}N nuclei at astrophysical energies

    SciTech Connect

    Dubovichenko, S. B.

    2013-07-15

    The possibility of describing experimental data on the total cross sections for the n{sup 2}H, n{sup 7}Li, n{sup 14}C, and n{sup 14}N radiative-capture processes within the potential cluster model involving forbidden states and their classification according to Young's tableaux is considered. It is shown that this model and the methods used here to construct potentials make it possible to describe correctly the behavior of the experimental cross sections at energies between 5 to 10 meV (5 Multiplication-Sign 10{sup -3}-10 Multiplication-Sign 10{sup -3} eV) and 1 to 15MeV.

  12. Trajectory-dependent resonant neutralization of low energy [sup 7]Li[sup +] scattered from clean and Na-covered Al(100)

    SciTech Connect

    German, K.A.H.; Weare, C.B.; Varekamp, P.R.; Yarmoff, J.A. Materials Sciences Division, Lawrence Berkeley Laboratory, Berkeley, California 94720 ); Andersen, J.N. )

    1993-07-01

    Trajectory-dependent neutralization is observed for low energy (1--5 keV) [sup 7]Li[sup +] ions scattered at large angles from Na-covered Al(100). Energy spectra and angular scans of the scattered Li[sup +] ion yield are collected as a function of Na coverage. Li[sup +] ions are partially neutralized upon single scattering from Al sites and completely neutralized when scattered from Na. This site-specific neutralization indicates that the surface electrostatic potential is nonuniform. The neutralization probability is also shown to be a function of the exit angle from the surface. The results are analyzed using theoretical ion fractions based on a semiclassical resonant charge exchange model.

  13. The influence of high-energy 7Li ions on the TL response and glow curve structure of CaSO4 : Dy

    NASA Astrophysics Data System (ADS)

    Salah, Numan; Sahare, P. D.

    2006-07-01

    Thermoluminescence (TL) of CaSO4 : Dy phosphor, irradiated by 48 MeV 7Li ions with different fluences in the range 1 × 109-5 × 1011 ions cm-2 has been studied. The samples from the same batch were also exposed to γ-rays from a Co60 source for comparative studies. The TL glow curve of the material, irradiated with the ion beam has a simple structure with a prominent peak at around 494 K along with three small shoulders at around 424, 592 and 662 K. The TL saturation has been observed at around the fluence 1 × 1011 ions cm-2. As the fluence is increased from 1 × 109 to 5 × 1011 ions cm-2, a shift in the peak positions towards the lower temperature side, by around 7 K was observed. However, with increasing fluence, the TL glow curve structure remains invariant with no change in the relative intensities between the 494 and 424 K peaks, while in the case of γ-irradiated samples, in contrast, the intensity ratios of these peaks increase exponentially with exposures. Theoretical analysis of the glow curves of the ion beam and γ-irradiated samples was done by the glow curve deconvolution method. The efficiency of CaSO4 : Dy to 48 MeV 7Li ions has been measured relative to γ-rays of Co60 and found to be 0.81. This result, along with the observed good linearity over a large span of fluences, shows that this phosphor is quite suitable as a dosimeter for heavy charged particles.

  14. Astrophysical S-factor of T(4He, γ)7Li reaction at E cm = 15.7 keV

    NASA Astrophysics Data System (ADS)

    Bystritsky, V. M.; Dudkin, G. N.; Emets, E. G.; Filipowicz, M.; Krylov, A. R.; Nechaev, B. A.; Nurkin, A.; Padalko, V. N.; Philippov, A. V.; Sadovsky, A. B.

    2017-07-01

    The astrophysical S-factor of the reaction T(4He, γ)7Li is measured for the first time at the center of mass energy E cm = 15.7 keV, lower than the energy range of the Standard Big Bang Nucleosynthesis (SBBN) model. The experiment is performed on a Hall pulsed accelerator (TPU, Tomsk). An acceleration pulse length of 10 μs allows one to suppress the background of cosmic radiation and the ambient medium by five orders of magnitude. A beam intensity of 5 × 1014 4He+ ions per pulse allows one to measure an extremely low reaction yield. The yield of γ-quanta with the energies E γ 0 = 2483.7 keV and E γ 1 = 2006.1 keV is registered by NaI(Tl) detectors with the efficiency ɛ = 0.331 ± 0.026. A method for direct measurement of the background from the chain of reactions T(4He, 4He)T→T(T, 2 n)X→( n, γ) and/or ( n, n'γ) which ends by neutron activation of materials surrounding the target is proposed and implemented in this study. The value of the astrophysical S-factor of the reaction T(4He, γ)7Li S αt ( E cm = 15.7 keV) = 0.091 ± 0.032 keV b provides the choice from the set of experimental data for the astrophysical S αt -factor in favor of experimental data [4] with S αt ( E cm = 0) = 0.1067 ± 0.0064 keV b.

  15. Relation of short-range and long-range lithium ion dynamics in glass-ceramics: Insights from 7Li NMR field-cycling and field-gradient studies

    NASA Astrophysics Data System (ADS)

    Haaks, Michael; Martin, Steve W.; Vogel, Michael

    2017-09-01

    We use various 7Li NMR methods to investigate lithium ion dynamics in 70Li 2S-30 P 2S5 glass and glass-ceramic obtained from this glass after heat treatment. We employ 7Li spin-lattice relaxometry, including field-cycling measurements, and line-shape analysis to investigate short-range ion jumps as well as 7Li field-gradient approaches to characterize long-range ion diffusion. The results show that ceramization substantially enhances the lithium ion mobility on all length scales. For the 70Li 2S-30 P 2S5 glass-ceramic, no evidence is found that bimodal dynamics result from different ion mobilities in glassy and crystalline regions of this sample. Rather, 7Li field-cycling relaxometry shows that dynamic susceptibilities in broad frequency and temperature ranges can be described by thermally activated jumps governed by a Gaussian distribution of activation energies g (Ea) with temperature-independent mean value Em=0.43 eV and standard deviation σ =0.07 eV . Moreover, use of this distribution allows us to rationalize 7Li line-shape results for the local ion jumps. In addition, this information about short-range ion dynamics further explains 7Li field-gradient results for long-range ion diffusion. In particular, we quantitatively show that, consistent with our experimental results, the temperature dependence of the self-diffusion coefficient D is not described by the mean activation energy Em of the local ion jumps, but by a significantly smaller apparent value whenever the distribution of correlation times G (logτ ) of the jump motion derives from an invariant distribution of activation energies and, hence, continuously broadens upon cooling. This effect occurs because the harmonic mean, which determines the results of diffusivity or also conductivity studies, continuously separates from the peak position of G (logτ ) when the width of this distribution increases.

  16. Astrophysical Impact of the Updated 9Be(p,α)6Li and 10B(p,α)7Be Reaction Rates As Deduced By THM

    NASA Astrophysics Data System (ADS)

    Lamia, L.; Spitaleri, C.; Tognelli, E.; Degl'Innocenti, S.; Pizzone, R. G.; Prada Moroni, P. G.

    2015-10-01

    The complete understanding of the stellar abundances of lithium, beryllium, and boron represents one of the most interesting open problems in astrophysics. These elements are largely used to probe stellar structure and mixing phenomena in different astrophysical scenarios, such as pre-main-sequence or main-sequence stars. Their different fragility against (p,α) burning reactions allows one to investigate different depths of the stellar interior. Such fusion mechanisms are triggered at temperatures between T ≈ (2-5) × {10}6 K, thus defining a corresponding Gamow energy between ≈ 3-10 keV, where S(E)-factor measurements need to be performed to get reliable reaction rate evaluations. The Trojan Horse Method is a well defined procedure to measure cross sections at Gamow energies overcoming the uncertainties due to low-energy S(E)-factor extrapolation as well as electron screening effects. Taking advantage of the {\\mathtt{THM}} measure of the 9Be(p,α)6Li and 10B(p,α)7Be cross sections, the corresponding reaction rates have been calculated and compared with the evaluations by the NACRE collaboration, widely used in the literature. The impact on surface abundances of the updated 9Be and 10B (p,α) burning rates is discussed for pre-MS stars.

  17. Pulse shape discrimination characteristics of stilbene crystal, pure and 6Li loaded plastic scintillators for a high resolution coded-aperture neutron imager

    NASA Astrophysics Data System (ADS)

    Cieślak, M. J.; Gamage, K. A. A.; Glover, R.

    2017-07-01

    Pulse shape discrimination performances of single stilbene crystal, pure plastic and 6Li loaded plastic scintillators have been compared. Three pulse shape discrimination algorithms have been tested for each scintillator sample, assessing their quality of neutron/gamma separation. Additionally, the digital implementation feasibility of each algorithm in a real-time embedded system was evaluated. Considering the pixelated architecture of the coded-aperture imaging system, a reliable method of simultaneous multi-channel neutron/gamma discrimination was sought, accounting for the short data analysis window available for each individual channel. In this study, each scintillator sample was irradiated with a 252Cf neutron source and a bespoke digitiser system was used to collect the data allowing detailed offline examination of the sampled pulses. The figure-of-merit was utilised to compare the discrimination quality of the collected events with respect to various discrimination algorithms. Single stilbene crystal presents superior neutron/gamma separation performance when compared to the plastic scintillator samples.

  18. Viscosity and carbon dioxide solubility for LiPF6, LiTFSI, and LiFAP in alkyl carbonates: lithium salt nature and concentration effect.

    PubMed

    Dougassa, Yvon Rodrigue; Jacquemin, Johan; El Ouatani, Loubna; Tessier, Cécile; Anouti, Mérièm

    2014-04-10

    In this paper, we have reported the CO2 solubility in different pure alkyl carbonate solvents (EC, DMC, EMC, DEC) and their binary mixtures as EC/DMC, EC/EMC, and EC/DEC and for electrolytes [solvent + lithium salt] LiX (X = LiPF6, LiTFSI, or LiFAP) as a function of the temperature and salt concentration. To understand the parameters that influence the structure of the solvents and their ability to dissolve CO2, through the addition of a salt, we first analyzed the viscosities of EC/DMC + LiX mixtures by means of a modified Jones-Dole equation. The results were discussed considering the order or disorder introduced by the salt into the solvent organization and ion solvation sphere by calculating the effective solute ion radius, rs. On the basis of these results, the analysis of the CO2 solubility variations with the salt addition was then evaluated and discussed by determining specific ion parameters Hi by using the Setchenov coefficients in solution. This study showed that the CO2 solubility has been affected by the shape, charge density, and size of the ions, which influence the structuring of the solvents through the addition of a salt and the type of solvation of the ions.

  19. Structure and reactivity of lithium amides. /sup 6/Li, /sup 13/C, and /sup 15/N NMR spectroscopic studies and colligative measurements of lithium diphenylamide and lithium diphenylamide-lithium bromide complex solvated by tetrahydrofuran

    SciTech Connect

    DePue, J.S.; Collum, D.B.

    1988-08-03

    /sup 6/Li, /sup 13/C, and /sup 15/N NMR spectroscopic studies of lithium diphenylamide in THF/hydrocarbon solutions (THF = tetrahydrofuran) detected two different species. /sup 6/Li and /sup 15/N NMR spectroscopic studies of (/sup 6/Li, /sup 15/N)lithium diphenylamide showed the species observed at low THF concentrations to be a cyclic oligomer. Structural analogies provided strong support for a dimer while colligative measurements at 0/degrees/C indicated the dimer to be di- or trisolvated. On the basis of the observed mass action effects, the species appearing at intermediate THF concentrations is assigned as a contact or solvent-separated ion-paired monomer. Lithium diphenylamide forms a 1:1 adduct with lithium bromide at low THF concentrations. A combination of /sup 6/Li-/sup 15/N double labeling studies and colligative measurements supports a trisolvated cyclic mixed dimer structure. Although detailed spectroscopic studies at elevated THF concentrations were precluded by high fluctionality, the similarity of the /sup 13/C chemical shifts of lithium diphenylamide in the presence and absence of lithium bromide provide indirect evidence that the mixed dimer undergoes a THF concentration dependent dissociation to the monomeric amide and free lithium bromide. 24 references, 9 figures, 2 tables.

  20. Computational, electrochemical and {sup 7}Li NMR studies of lithiated disordered carbons electrodes in lithium ion cells.

    SciTech Connect

    Sandi, G.; Gerald, R., II; Scanlon, L. G.; Carrado, K. A.; Winans, R. E.

    1998-01-07

    Disordered carbons that deliver high reversible capacity in electrochemical cells have been synthesized by using inorganic clays as templates to control the pore size and the surface area. The capacities obtained were much higher than those calculated if the resultant carbon had a graphitic-like structure. Computational chemistry was used to investigate the nature of lithium bonding in a carbon lattice unlike graphite. The lithium intercalated fullerene Li{sub n}-C{sub 60} was used as a model for our (non-graphitic) disordered carbon lattice. A dilithium-C{sub 60} system with a charge and multiplicity of (0,1) and a trilithium-C{sub 60} system with a charge and multiplicity of (0,4) were investigated. The spatial distribution of lithium ions in an electrochemical cell containing this novel disordered carbon material was investigated in situ by Li-7 NMR using an electrochemical cell that was incorporated into a toroid cavity nuclear magnetic resonance (NMR) imager. The concentration of solvated Li{sup +} ions in the carbon anode appears to be larger than in the bulk electrolyte, is substantially lower near the copper/carbon interface, and does not change with cell charging.

  1. 6-Li enriched Cs2LiYCl6:Ce based thermal neutron detector coupled with CMOS solid-state photomultipliers for a portable detector unit

    NASA Astrophysics Data System (ADS)

    Whitney, Chad; Stapels, Christopher; Johnson, Erik; Chapman, Eric; Alberghini, Guy; Glodo, Jarek; Shah, Kanai; Christian, James

    2011-03-01

    For detecting neutrons, 3-He tubes provide sensitivity and a unique capability for detecting and discriminating neutron signals from background gamma-ray signals. A solid-state scintillation-based detector provides an alternative to 3-He for neutron detection. A real-time, portable, and low cost thermal neutron detector has been constructed from a 6Li-enriched Cs2LiYCl6:Ce (CLYC) scintillator crystal coupled with a CMOS solid-state photomultiplier (SSPM). These components are fully integrated with a miniaturized multi-channel analyzer (MCA) unit for calculation and readout of the counts and count rates. CLYC crystals and several other elpasolites including Cs2LiLaCl6:Ce (CLLC) and Cs2LiLaBr6:Ce (CLLB) have been considered for their unique properties in detecting neutrons and discriminating gamma ray events along with providing excellent energy resolution comparable to NaI(Tl) scintillators. CLYC's slower rise and decay time for neutrons (70ns and 900ns respectively) relative to a faster rise and decay time for gamma ray events (6ns and 55ns respectively) allows for pulse shape discrimination in mixed radiation fields. Light emissions from CLYC crystals are detected using an array of avalanche photodiodes referred to as solid-state photomultipliers. SSPMs are binary photon counting devices where the number of pixels activated is directly proportional to the light output of the CLYC scintillator which is proportional to the energy deposited from the radiation field. SSPMs can be fabricated using standard CMOS processes and inherently contain the low noise performance associated with ordinary photomultiplier tubes (PMT) while providing a light and compact solution for portable neutron detectors.

  2. Diffraction dissociation of {sup 7}Li and {sup 7}Be relativistic nuclei on proton targets through the {sup 3}H({sup 3}He)+{sup 4}He channels

    SciTech Connect

    Fetisov, V. N.

    2015-07-15

    For the fragmentation of {sup 7}Li and {sup 7}Be relativistic nuclei (with momenta of, respectively, P = 3 GeV/c and P = 1.6 GeV/c per nucleon) on proton targets through the {sup 3}H({sup 3}He) + {sup 4}He channels, the differential cross sections with respect to the momentum transfer Q to the fragments were calculated on the basis of the cluster version of Akhiezer–Glauber–Sitenko diffraction theory by employing the twobody cluster model for the {sup 7}Li ({sup 3}H + {sup 4}He) and {sup 7}Be ({sup 3}He + {sup 4}He) nuclei. These calculations, performed in the impulse approximation in the interaction of intranuclear clusters with the target nucleus, explained a strong suppression of the cross sections for reactions on protons at Q lower than 100 MeV/c and higher than 350 MeV/c and the observed irregularities in the behavior off the cross section for {sup 7}Li fragmentation on complex track-emulsion nuclei. Cross-section values close to their experimental counterparts were obtained upon setting the coefficient of two-body clustering in the {sup 7}Li and {sup 7}Be nuclei to k ≃ 0.7.

  3. Microdosimetry measurements characterizing the radiation fields of 300 MeV/u 12C and 185 MeV/u 7Li pencil beams stopping in water.

    PubMed

    Martino, G; Durante, M; Schardt, D

    2010-06-21

    In order to characterize the complex radiation field produced by heavy-ion beams in water, in particular the lateral dose fall-off and the radiation quality, microdosimetry measurements were performed at GSI Darmstadt using pencil-like beams of 300 MeV/u (12)C and 185 MeV/u (7)Li ions delivered by the heavy-ion synchrotron SIS-18. The ion beams (range in water about 17 cm) were stopped in the center of a 30 x 30 x 30 cm(3) water phantom and their radiation field was investigated by in-phantom measurements using a tissue-equivalent proportional chamber (TEPC). The chamber was placed at 35 different positions in the central plane at various depths along the beam axis and at radial distances of 0, 1, 2, 5 and 10 cm. The off-axis measurements for both (12)C and (7)Li ions show very similar distributions of the lineal energy, all peaking between 1 and 10 keV microm(-1) which is a typical range covered by secondary hydrogen fragments and neutrons. The radiation quality given by the dose-mean lineal energy [Formula in text] was found to be at a constant level of 1-2 keV microm(-1) at radial distances larger than 2 cm. The relative absorbed dose at each position was obtained by integration of the measured spectra normalized to the number of incident primary beam particles. The results confirm that the lateral dose profile of heavy ions shows an extremely steep fall-off, with relative values of about 10(-3), 10(-4) and 10(-5) at the 2, 5 and 10 cm distance from the beam axis, respectively. The depth-dose curves at a fixed distance from the beam axis slowly rise until they reach the depth of the Bragg peak, reflecting the build-up of secondary fragments with increasing penetration depth. The measured (12)C dose profiles were found to be in good agreement with a similar experimental study at HIMAC (Japan).

  4. Ultracold Collisions Involving Heteronuclear Alkali Metal Dimers

    SciTech Connect

    Cvitas, Marko T.; Soldan, Pavel; Hutson, Jeremy M.; Honvault, Pascal; Launay, Jean-Michel

    2005-05-27

    We carry out the first quantum dynamics calculations on ultracold atom-diatom collisions in isotopic mixtures. The systems studied are spin-polarized {sup 7}Li+{sup 6}Li{sup 7}Li, {sup 7}Li+{sup 6}Li{sub 2}, {sup 6}Li+{sup 6}Li{sup 7}Li, and {sup 6}Li+{sup 7}Li{sub 2}. Reactive scattering can occur for the first two systems even when the molecules are in their ground rovibrational states, but is slower than vibrational relaxation in homonuclear systems. Implications for sympathetic cooling of heteronuclear molecules are discussed.

  5. A microdosimetric study of {sup 10}B(n,{alpha}){sup 7}Li and {sup 157}Gd(n,{gamma}) reactions for neutron capture therapy

    SciTech Connect

    Wang, C.K.C.; Sutton, M.; Evans, T.M.; Laster, B.H.

    1999-01-01

    This paper presents the microdosimetric analysis for the most interesting cell survival experiment recently performed at the Brookhaven National Laboratory (BNL). In this experiment, the cells were first treated with a gadolinium (Gd) labeled tumor-seeking boronated porphyrin (Gd-BOPP) or with BOPP alone, and then irradiated with thermal neutrons. The resulting cell-survival curves indicate that the {sup 157}Gd(n,{gamma}) reactions are very effective in cell killing. The death of a cell treated with Gd-BOPP was attributed to either the {sup 10}B(n,{alpha}){sup 7}Li reactions or the {sup 157}Gd(n,{gamma}) reactions (or both). However, the quantitative relationship between the two types of reaction and the cell-survival fraction was not clear. This paper presents the microdosimetric analysis for the BNL experiment based on the measured experimental parameters, and the results clearly suggest a quantitative relationship between the two types of reaction and the cell survival fraction. The results also suggest new research in gadolinium neutron capture therapy (GdNCT) which may lead to a more practical modality than the boron neutron capture therapy (BNCT) for treating cancers.

  6. Ab initio structure search and in situ 7Li NMR studies of discharge products in the Li–S battery system

    DOE PAGES

    See, Kimberly A.; Leskes, Michal; Griffin, John M.; ...

    2014-11-10

    The high theoretical gravimetric capacity of the Li–S battery system makes it an attractive candidate for numerous energy storage applications. In practice, cell performance is plagued by low practical capacity and poor cycling. In an effort to explore the mechanism of the discharge with the goal of better understanding performance, we examine the Li–S phase diagram using computational techniques and complement this with an in situ 7Li NMR study of the cell during discharge. Both the computational and experimental studies are consistent with the suggestion that the only solid product formed in the cell is Li2S, formed soon after cellmore » discharge is initiated. In situ NMR spectroscopy also allows the direct observation of soluble Li+-species during cell discharge; species that are known to be highly detrimental to capacity retention. We suggest that during the first discharge plateau, S is reduced to soluble polysulfide species concurrently with the formation of a solid component (Li2S) which forms near the beginning of the first plateau, in the cell configuration studied here. The NMR data suggest that the second plateau is defined by the reduction of the residual soluble species to solid product (Li2S). Lastly, a ternary diagram is presented to rationalize the phases observed with NMR during the discharge pathway and provide thermodynamic underpinnings for the shape of the discharge profile as a function of cell composition.« less

  7. Development of liquid-lithium film jet-flow for the target of (7)Li(p,n)(7)Be reactions for BNCT.

    PubMed

    Kobayashi, Tooru; Miura, Kuniaki; Hayashizaki, Noriyosu; Aritomi, Masanori

    2014-06-01

    A feasibility study on liquid lithium target in the form of a flowing film was performed to evaluate its potential use as a neutron generation target of (7)Li(p,n)(7)Be reaction in BNCT. The target is a windowless-type flowing film on a concave wall. Its configuration was adapted for a proton beam which is 30mm in diameter and with energy and current of up to 3MeV and 20mA, respectively. The flowing film of liquid lithium was 0.6mm in thickness, 50mm in width and 50mm in length. The shapes of the nozzle and concave back wall, which create a stable flowing film jet, were decided based on water experiments. A lithium hydrodynamic experiment was performed to observe the stability of liquid lithium flow behavior. The flowing film of liquid lithium was found to be feasible at temperatures below the liquid lithium boiling saturation of 342°C at the surface pressure of 1×10(-3)Pa. Using a proto-type liquid lithium-circulating loop for BNCT, the stability of the film flow was confirmed for velocities up to 30m/s at 220°C and 250°C in vacuum at a pressure lower than 10(-3) Pa. It is expected that for practical use, a flowing liquid lithium target of a windowless type can solve the problem of radiation damage and target cooling.

  8. Formation of ultracold {sup 7}Li{sup 85}Rb molecules in the lowest triplet electronic state by photoassociation and their detection by ionization spectroscopy

    SciTech Connect

    Altaf, Adeel Dutta, Sourav; Lorenz, John; Pérez-Ríos, Jesús; Chen, Yong P.; Elliott, D. S.

    2015-03-21

    We report the formation of ultracold {sup 7}Li{sup 85}Rb molecules in the a{sup 3}Σ{sup +} electronic state by photoassociation (PA) and their detection via resonantly enhanced multiphoton ionization (REMPI). With our dual-species Li and Rb magneto-optical trap apparatus, we detect PA resonances with binding energies up to ∼62 cm{sup −1} below the {sup 7}Li 2s {sup 2}S{sub 1/2} + {sup 85}Rb 5p {sup 2}P{sub 1/2} asymptote. In addition, we use REMPI spectroscopy to probe the a{sup 3}Σ{sup +} state and excited electronic 3{sup 3}Π and 4{sup 3}Σ{sup +} states and identify a{sup 3}Σ{sup +} (v″ = 7–13), 3{sup 3}Π (v{sub Π}′ = 0–10), and 4{sup 3}Σ{sup +} (v{sub Σ}′ = 0–5) vibrational levels. Our line assignments agree well with ab initio calculations. These preliminary spectroscopic studies on previously unobserved electronic states are crucial to discovering transition pathways for transferring ultracold LiRb molecules created via PA to deeply bound rovibrational levels of the electronic ground state.

  9. What is the best proton energy for accelerator-based BNCT using the 7Li(p,n)7Be reaction?

    PubMed

    Allen, D A; Beynon, T D

    2000-05-01

    With a growing interest in the use of accelerator-based epithermal neutron sources for BNCT programs, in particular those based upon the 7Li(p,n)7Be reaction, there is a need to address the question of "what is the best proton energy to use?" This paper considers this question by using radiation transport calculations to investigate a range of proton energies from 2.15 to 3.5 MeV and a range of moderator sizes. This study has moved away completely from the use of empty therapy beam parameters and instead defines the beam quality and optimizes the moderator design using widely accepted in-phantom treatment planning figures of merit. It is concluded that up to a proton energy of about 2.8 MeV there is no observed variation in the achievable therapy beam quality, but a price is paid in terms of treatment time for not choosing the upper limit of this range. For higher proton energies, the beam quality falls, but with no improvement in treatment time for optimum configurations.

  10. A microdosimetric study of {sup 10}B(n,{alpha}){sup 7}Li and {sup 157}Gd(n,{gamma}) reactions for neutron capture therapy

    SciTech Connect

    Wang, C.K.C.; Sutton, M.; Evans, T.M.; Laster, B.H.

    1996-12-31

    This paper presents the microdosimetric analysis for the most interesting cell survival experiment recently performed at the Brookhaven National Laboratory (BNL). In this experiment, the cells were first treated with a gadolinium (Gd) labeled tumor-seeking boronated porphyrin (Gd-BOPP) or with BOPP alone, and then irradiated with thermal neutrons. The resulting cell survival curves indicate that the {sup 157}Gd(n,{gamma}) reactions is very effective in cell killing. The death of a cell treated with GD-BOPP were attributed to either the {sup 10}B(n,{alpha}) {sup 7}Li reactions or the {sup 157}Gd(n,{gamma}) reactions (or both). However, the quantitative relationship between the two types of reaction and the cell survival fraction was not clear. This paper presents the microdosimetric analysis for the BNL experiment based on the measured experimental parameters, and the results clearly suggest a quantitative relationship between the two types of reaction and the cell survival fraction. The results also suggest new research in Gadolinium neutron capture therapy (GDNCT) which may lead to a more practical modality than the boron neutron capture therapy (BNCT) for treating cancers.

  11. Nuclear Astrophysics and Structure Studies Using Low-energy RI Beams at CRIB

    SciTech Connect

    Yamaguchi, H.; Hashimoto, T.; Hayakawa, S.; Binh, D. N.; Kahl, D.; Kubono, S.

    2010-05-12

    CRIB (CNS Radioactive Ion Beam separator) is a low-energy RI beam separator at the Center for Nuclear Study (CNS) of the University of Tokyo. Using the RI beams at CRIB, Many measurements on proton and alpha resonance scatterings, (alpha,p) reactions, and others were peformed in recent years, mainly for studying astrophysical reactions and exotic nuclear structure. Among them, the results on the {sup 7}Be+p and {sup 7}Li+alpha resonance scatterings are presented.

  12. Theoretical nuclear physics

    SciTech Connect

    Kunz, P.D.

    1990-10-01

    This report contains small papers on the following topics: ground state correlations of nuclei in relativistic random phase approximation; instability of infinite nuclear matter in the relativistic hartree approximation; charge density differences for nuclei near {sup 208}Pb in relativistic models; meson exchange current corrections to magnetic moments in quantum hadro-dynamics; analysis of the O{sup +} {yields} O{sup {minus}} reaction at intermediate energies; contributions of reaction channels to the {sup 6}Li(p,{gamma}){sup 7}Be Reaction; deformed chiral nucleons; vacuum polarization in a finite system; second order processes in the (e,e{prime}d) reaction; sea contributions in Dirac RPA for finite nuclei; and momentum cutoffs in the sea.

  13. Near-threshold (7)Li(p,n)(7)Be neutrons on the practical conditions using thick Li-target and Gaussian proton energies for BNCT.

    PubMed

    Kobayashi, Tooru; Hayashizaki, Noriyosu; Katabuchi, Tatsuya; Tanaka, Kenichi; Bengua, Gerard; Nakao, Noriaki; Kosako, Kazuaki

    2014-06-01

    The near threshold (7)Li(p,n)(7)Be neutrons generated by incident proton energy having Gaussian distribution with mean energies from 1.85 to 1.95MeV, were studied as a practical neutron source for BNCT wherein an RFQ accelerator and a thick Li-target are used. Gaussian energy distributions with the standard deviation of 0, 10, 20 and 40keV for mean proton energies from 1.85 to 1.95MeV were surveyed in 0.01MeV increments. A thick liquid Li-target whose dimensions were established in our previous experiments (i.e., 1mm-thick with 50mm width and 50mm length) was considered in this study. The suitable incident proton energy and physical dimensions of Pb layer which serves as a gamma absorber and a Polyethylene layer which is used as a BDE were surveyed by means of the concepts of TPD. Dose distribution were calculated by using MCNP5. A proton beam with mean energy of 1.92MeV and a Gaussian energy distribution with a standard deviation of 20keV at a current of 10mA was selected from the viewpoint of irradiation time and practically achievable proton current. The suitable thicknesses of Pb gamma absorber was estimated to be about 3cm. The estimated thickness of the polyethylene BDE was about 24mm for an ideal proton current of 13mA, and was 18mm for a practical proton current of 10mA.

  14. Experimental differential cross sections, level densities, and spin cutoffs as a testing ground for nuclear reaction codes

    DOE PAGES

    Voinov, Alexander V.; Grimes, Steven M.; Brune, Carl R.; ...

    2013-11-08

    Proton double-differential cross sections from 59Co(α,p)62Ni, 57Fe(α,p)60Co, 56Fe(7Li,p)62Ni, and 55Mn(6Li,p)60Co reactions have been measured with 21-MeV α and 15-MeV lithium beams. Cross sections have been compared against calculations with the empire reaction code. Different input level density models have been tested. It was found that the Gilbert and Cameron [A. Gilbert and A. G. W. Cameron, Can. J. Phys. 43, 1446 (1965)] level density model is best to reproduce experimental data. Level densities and spin cutoff parameters for 62Ni and 60Co above the excitation energy range of discrete levels (in continuum) have been obtained with a Monte Carlo technique. Furthermore,more » excitation energy dependencies were found to be inconsistent with the Fermi-gas model.« less

  15. Experimental differential cross sections, level densities, and spin cutoffs as a testing ground for nuclear reaction codes

    NASA Astrophysics Data System (ADS)

    Voinov, A. V.; Grimes, S. M.; Brune, C. R.; Bürger, A.; Görgen, A.; Guttormsen, M.; Larsen, A. C.; Massey, T. N.; Siem, S.

    2013-11-01

    Proton double-differential cross sections from 59Co(α,p)62Ni, 57Fe(α,p)60Co, 56Fe(7Li,p)62Ni, and 55Mn(6Li,p)60Co reactions have been measured with 21-MeV α and 15-MeV lithium beams. Cross sections have been compared against calculations with the empire reaction code. Different input level density models have been tested. It was found that the Gilbert and Cameron [A. Gilbert and A. G. W. Cameron, Can. J. Phys.0008-420410.1139/p65-139 43, 1446 (1965)] level density model is best to reproduce experimental data. Level densities and spin cutoff parameters for 62Ni and 60Co above the excitation energy range of discrete levels (in continuum) have been obtained with a Monte Carlo technique. Excitation energy dependencies were found to be inconsistent with the Fermi-gas model.

  16. Neutronic data in support of space nuclear propulsion

    SciTech Connect

    Mughabghab, S.; Schmidt, E.; Ludewig, H.

    1997-07-01

    The thermophysical properties of lithium hydride ({sup 7}LiH), particularly small density (0.775 gm/cc), high melting point (688 C) and relatively high hydrogen atomic number density makes it an attractive material for use as a neutron moderator and shield (for LiH) in space nuclear thermal propulsion. However, the unavailability of neutronic cross section data in the thermal energy range for {sup 7}LiH in the ENDF/B library necessitated the generation of the relevant data which is required in criticality studies and for the determination of temperature-dependent feedback coefficients in the moderator and fuel regions. Here, the scattering kernel data for {sup 7}LiH have been generated for the first time in the temperature range 50--1,000 K. This is based on a phonon distribution function derived from both experimental data and theoretical calculations. A detailed study of the variation of the moderator temperature coefficient {alpha}{sub m}(T) with temperature, T, is carried out for a typical space nuclear reactor of the particle bed type. It is established that the moderator temperature coefficient is proportional to T{sup {minus}1.65} where T is the moderator temperature in Kelvin units.

  17. Competition between Na + and Li + for Unsealed and Cytoskeleton-Depleted Human Red Blood Cell Membrane: A 23Na Multiple Quantum Filtered and 7Li NMR Relaxation Study

    NASA Astrophysics Data System (ADS)

    Srinivasan, Chandra; Minadeo, Nicole; Toon, Jason; Graham, Daniel; Mota de Freitas, Duarte; Geraldes, Carlos F. G. C.

    1999-09-01

    Evidence for competition between Li+ and Na+ for binding sites of human unsealed and cytoskeleton-depleted human red blood cell (csdRBC) membranes was obtained from the effect of added Li+ upon the 23Na double quantum filtered (DQF) and triple quantum filtered (TQF) NMR signals of Na+-containing red blood cell (RBC) membrane suspensions. We found that, at low ionic strength, the observed quenching effect of Li+ on the 23Na TQF and DQF signal intensity probed Li+/Na+ competition for isotropic binding sites only. Membrane cytoskeleton depletion significantly decreased the isotropic signal intensity, strongly affecting the binding of Na+ to isotropic membrane sites, but had no effect on Li+/Na+ competition for those sites. Through the observed 23Na DQF NMR spectra, which allow probing of both isotropic and anisotropic Na+ motion, we found anisotropic membrane binding sites for Na+ when the total ionic strength was higher than 40 mM. This is a consequence of ionic strength effects on the conformation of the cytoskeleton, in particular on the dimer-tetramer equilibrium of spectrin. The determinant involvement of the cytoskeleton in the anisotropy of Na+ motion at the membrane surface was demonstrated by the isotropy of the DQF spectra of csdRBC membranes even at high ionic strength. Li+ addition initially quenched the isotropic signal the most, indicating preferential Li+/Na+ competition for the isotropic membrane sites. High ionic strength also increased the intensity of the anisotropic signal, due to its effect on the restructuring of the membrane cytoskeleton. Further Li+ addition competed with Na+ for those sites, quenching the anisotropic signal. 7Li T1 relaxation data for Li+-containing suspensions of unsealed and csdRBC membranes, in the absence and presence of Na+ at low ionic strength, showed that cytoskeleton depletion does not affect the affinity of Na+ for the RBC membrane, but increases the affinity of Li+ by 50%. This clearly indicates that cytoskeleton

  18. Folding model analysis of 240 MeV {sup 6}Li elastic scattering on {sup 116}Sn and inelastic scattering to low-lying states of {sup 116}Sn

    SciTech Connect

    Chen, X.; Lui, Y.-W.; Clark, H. L.; Tokimoto, Y.; Youngblood, D. H.

    2007-11-15

    Elastic scattering of 240 MeV {sup 6}Li ions from {sup 116}Sn was measured from 4 deg.{<=}{theta}{sub c.m.}{<=}32 deg. The data were fitted with a Woods-Saxon phenomenological potential and with double folding models using the M3Y NN effective interaction with and without density dependence. DWBA calculations with the fitted parameters were used to calculate cross sections for inelastic scattering to low-lying 2{sup +}and 3{sup -} states. B(E2) and B(E3) values were extracted and compared with electromagnetic values and those obtained from {alpha} inelastic scattering.

  19. Ca(AlH4)2, CaAlH5, and CaH2+6LiBH4: Calculated dehydrogenation enthalpy, including zero point energy, and the structure of the phonon spectra.

    PubMed

    Marashdeh, Ali; Frankcombe, Terry J

    2008-06-21

    The dehydrogenation enthalpies of Ca(AlH(4))(2), CaAlH(5), and CaH(2)+6LiBH(4) have been calculated using density functional theory calculations at the generalized gradient approximation level. Harmonic phonon zero point energy (ZPE) corrections have been included using Parlinski's direct method. The dehydrogenation of Ca(AlH(4))(2) is exothermic, indicating a metastable hydride. Calculations for CaAlH(5) including ZPE effects indicate that it is not stable enough for a hydrogen storage system operating near ambient conditions. The destabilized combination of LiBH(4) with CaH(2) is a promising system after ZPE-corrected enthalpy calculations. The calculations confirm that including ZPE effects in the harmonic approximation for the dehydrogenation of Ca(AlH(4))(2), CaAlH(5), and CaH(2)+6LiBH(4) has a significant effect on the calculated reaction enthalpy. The contribution of ZPE to the dehydrogenation enthalpies of Ca(AlH(4))(2) and CaAlH(5) calculated by the direct method phonon analysis was compared to that calculated by the frozen-phonon method. The crystal structure of CaAlH(5) is presented in the more useful standard setting of P2(1)c symmetry and the phonon density of states of CaAlH(5), significantly different to other common complex metal hydrides, is rationalized.

  20. Polarization observables in [pi][sup +] [sup 6]Li scattering: Analyzing powers [ital iT][sub 11] and [tau][sub 22

    SciTech Connect

    Ritt, S.; Boschitz, E.; Brinkmoeller, B.; Buehler, J.; Meier, R.; Wessler, M. ); Konter, J.A.; Mango, S.; van den Brandt, B. ); Kamalov, S.S. ); Eramzhyan, R.A. ); Ryzhikh, G.G. )

    1994-06-01

    The vector analyzing power [ital iT][sub 11] and the tensor analyzing power [tau][sub 22]=[ital T][sub 22]+[ital T][sub 20]/ [radical]6 have been measured for [pi][sup +][r arrow][sup 6]L[rvec i] elastic and inelastic scattering (to the 3[sup +]0, 2.19 MeV state) at incident pion energies of 120, 150, 180, and 194 MeV. These data and earlier ones from our group are compared with new coupled channels calculations. Within the coupled channels model, the influence of different nuclear wave functions, the strength of the coupling of the ground and first excited states, and the effects of the phenomenological second-order potential were investigated. It was found that the calculated vector analyzing power [ital iT][sub 11] depends strongly on the transverse form factor whichever nuclear wave function is chosen. In the angular region where the [ital iT][sub 11] data were taken the coupling of the ground to the first excited state has a minor effect on the theoretical predictions. Reasonable agreement with the data can be obtained for a large energy and angular region with the first-order potential only.

  1. Measurements of the neutron yields from 7Li(p,n)7Be reaction (thick target) with incident energies from 1.885 to 2.0 MeV.

    PubMed

    Yu, W; Yue, G; Han, X; Chen, J; Tian, B

    1998-07-01

    Accelerator-based neutron source have been considered to be practical for boron neutron capture therapy (BNCT). Based on experience with a parameters of the Brookhaven National Laboratory BMRR reactor neutron source, which has been used in treatment experiments, the future accelerator-based neutron source for BNCT should have the properties of low energy distribution (< 100 keV) and high flux (about 10(9) neutrons per second per square centimeter) in the patient zone. Using protons to bombard thick 7Li targets, generating neutrons via the 7Li(p,n)7Be reaction, is one of the optimal choices for this kind of neutron source. Neutron yield data versus incident energy are necessary in order to select the proper incident energy and for estimating how high the incident proton current should be. The required proton beam current intensity is one of the key parameters for an accelerator useful for BNCT. In the present work, neutron yields of the 7Li(p,n)7Be reaction with a thick lithium target and incident energies of 1.885 and 1.9 MeV were measured at 0 degree with respect to the incident beam direction. The results are (3.08 +/- 0.17) x 10(12) and (5.71 +/- 0.32) x 10(12) neutrons/C sr, respectively. Neutron yield angular distribution measurements at 2 MeV incident energy were also performed. The proton beams were generated by the Peking University 4.5 MV electrostatic accelerator. The emitted neutrons from these reactions have the advantages of low energy distribution and forward angular distribution, which are requirements for a BNCT neutron source. The data obtained in this work can be used as a reference to study the accelerator-based neutron sources for BNCT.

  2. Report to the DOE Nuclear Data Committee, 1985

    SciTech Connect

    White, R.M.; Lanier, R.G.

    1985-02-01

    Progress is reported on the following measurements: the leakage multiplication from hollow beryllium spheres; /sup 6/Li and /sup 7/Li neutron-induced tritium production cross sections at 15 MeV; fast neutron fission yields; /sup 238/U(t,X) cross sections; neutron capture cross sections for /sup 86/ /sup 87/Sr at stellar temperatures; influence of realistic single particle spacings on precompound decay spectra; spontaneous fissions from a source of /sup 260/Md; and excitation functions from proton and deutron bombardment of natural Ti. Progress on the following calculations are reported: using modeled discrete levels; modeling level structures of odd-odd deformed nuclei; test of a phenomenological model of odd-odd deformed nuclei (an ARC study of /sup 176/Lu); absolute dipole gamma-ray strength functions for /sup 176/Lu; Gamow-Teller matrix elements for the /sup 11/B(p,n)/sup 11/C reaction at Ep = 26 MeV; K-distribution for neutron fission of /sup 232/Th; shell model study of the /sup 71/Ga(nu, anti e)/sup 71/Ge neutrino detector; and extension of microscopic models for neutron and proton scattering to inelastic scattering and charge-exchange reactions. Also, the status of the re-evaluation of the /sup 9/Be(n, 2n) reaction is given. (WHK)

  3. Effect of nuclear-reaction mechanisms on the population of excited nuclear states and isomeric ratios

    SciTech Connect

    Skobelev, N. K.

    2016-07-15

    Experimental data on the cross sections for channels of fusion and transfer reactions induced by beams of radioactive halo nuclei and clustered and stable loosely bound nuclei were analyzed, and the results of this analysis were summarized. The interplay of the excitation of single-particle states in reaction-product nuclei and direct reaction channels was established for transfer reactions. Respective experiments were performed in stable ({sup 6}Li) and radioactive ({sup 6}He) beams of the DRIBs accelerator complex at the Flerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, and in deuteron and {sup 3}He beams of the U-120M cyclotron at the Nuclear Physics Institute, Academy Sciences of Czech Republic (Řež and Prague, Czech Republic). Data on subbarrier and near-barrier fusion reactions involving clustered and loosely bound light nuclei ({sup 6}Li and {sup 3}He) can be described quite reliably within simple evaporation models with allowance for different reaction Q-values and couple channels. In reactions involving halo nuclei, their structure manifests itself most strongly in the region of energies below the Coulomb barrier. Neutron transfer occurs with a high probability in the interactions of all loosely bound nuclei with light and heavy stable nuclei at positive Q-values. The cross sections for such reactions and the respective isomeric ratios differ drastically for nucleon stripping and nucleon pickup mechanisms. This is due to the difference in the population probabilities for excited single-particle states.

  4. Effect of nuclear-reaction mechanisms on the population of excited nuclear states and isomeric ratios

    NASA Astrophysics Data System (ADS)

    Skobelev, N. K.

    2016-07-01

    Experimental data on the cross sections for channels of fusion and transfer reactions induced by beams of radioactive halo nuclei and clustered and stable loosely bound nuclei were analyzed, and the results of this analysis were summarized. The interplay of the excitation of single-particle states in reaction-product nuclei and direct reaction channels was established for transfer reactions. Respective experiments were performed in stable (6Li) and radioactive (6He) beams of the DRIBs accelerator complex at the Flerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, and in deuteron and 3He beams of the U-120M cyclotron at the Nuclear Physics Institute, Academy Sciences of Czech Republic (Řež and Prague, Czech Republic). Data on subbarrier and near-barrier fusion reactions involving clustered and loosely bound light nuclei (6Li and 3He) can be described quite reliably within simple evaporation models with allowance for different reaction Q-values and couple channels. In reactions involving halo nuclei, their structure manifests itself most strongly in the region of energies below the Coulomb barrier. Neutron transfer occurs with a high probability in the interactions of all loosely bound nuclei with light and heavy stable nuclei at positive Q-values. The cross sections for such reactions and the respective isomeric ratios differ drastically for nucleon stripping and nucleon pickup mechanisms. This is due to the difference in the population probabilities for excited single-particle states.

  5. Measurement of the parity-violating asymmetry in the reactions of cold polarized neutrons and light nuclei 6Li, 10B

    NASA Astrophysics Data System (ADS)

    Vesna, V. A.; Gledenov, Yu. M.; Nesvizhevsky, V. V.; Petukhov, A. K.; Sedyshev, P. V.; Soldner, T.; Shulgina, E. V.

    2009-08-01

    We present two measurements of parity-violating secondary particle emission asymmetry in the reactions of polarized cold neutrons and light nuclei. We aim at studies of the neutral weak currents in nucleon-nucleon interaction. First, we describe the triton emission asymmetry in the Li6(n,α)H3 reaction. It is equal to αP-odd6=-(8.8±2.1)ṡ10. Second, we present the γ-rays emission asymmetry in the nuclear reaction B10(n,α)Li∗7→γ→Li7(g.s.). The result is αP-odd10=+(0.8±3.9)ṡ10. Using these values, we constrain the weak neutral current constant in framework of the cluster model fπ6⩽1.1ṡ10 and fπ10⩽2.4ṡ10 (at 90% c.i.). Both these constrains contradict to “the best” DDH value of fπDDH=4.6ṡ10.

  6. A solution to lithium problem by long-lived stau

    NASA Astrophysics Data System (ADS)

    Sato, Joe; Shimomura, Takashi; Yamanaka, Masato

    We review a nonstandard Big-Bang Nucleosynthesis (BBN) scenario within the minimal supersymmetric standard model, and propose an idea to solve both the 7Li and 6Li problems. Each problem is a discrepancy between the predicted abundance in the standard BBN and observed one. We focus on the stau, a supersymmetric partner of tau lepton, which is a long-lived charged particle when it is the next lightest supersymmetric particle and is degenerate in mass with the lightest supersymmetric particle. The long-lived stau forms a bound state with a nucleus, and provides nonstandard nuclear reactions. One of those, the internal conversion process, accelerates the destruction of 7Be and 7Li, and leads to a solution to the 7Li problem. On the other hand, the bound state of the stau and 4He enhances productions of n, D, T and 6Li. The over-production of 6Li could solve the 6Li problem; while the over-productions of D and T could conflict with observations, and hence the relevant parameter space of the stau is strictly constrained. We therefore need to carefully investigate the stau-4He bound state to find a condition of solving the 6Li problem. The scenario of the long-lived stau simultaneously and successfully fits the abundances of light elements (D, T, 3He, 4He, 6Li and 7Li) and the neutralino dark matter to the observed ones. Consequently, the parameter space both of the stau and the neutralino is determined with excellent accuracy.

  7. Study of structure of nuclei with neutrons and nuclear data measurements for MFE. Progress report, September 1, 1979-August 31, 1980

    SciTech Connect

    Lane, R. O.

    1980-01-01

    Measurements of neutron differential elastic and inelastic scattering cross sections have been made for /sup 6/Li, /sup 7/Li, /sup 11/B and /sup 13/C. For /sup 7/Li + n, a multichannel R-matrix analysis has been completed, providing much new structure information for the compound /sup 8/Li system. These results are in very good agreement with recent theoretical model calculations, so that together the two provide considerable advancement in the state of our knowledge of /sup 8/Li. R-matrix analyses of /sup 11/B + n and /sup 13/C + n elastic scattering data have also been completed. For /sup 13/C + n theoretical model calculations have also been carried out and comparisons of these theoretical results with the R-matrix analysis are made. The triplet quadrupole spectrometer (TQS) is now fully operational. Development of new detectors, techniques, data analysis codes and theoretical model codes for use with the TQS system is complete. Measurements of (n,z) cross sections for fusion reactor structural materials e.g. /sup 58/Ni are currently underway. Construction of the long-flight-path tunnel for the swinger magnet facility has begun and development for this facility will continue in the coming year.

  8. Dose distributions in a human head phantom for neutron capture therapy using moderated neutrons from the 2.5 meV proton-7Li reaction or from fission of 235U.

    PubMed

    Tanaka, K; Kobayashi, T; Sakurai, Y; Nakagawa, Y; Endo, S; Hoshi, M

    2001-10-01

    The feasibility of neutron capture therapy (NCT) using an accelerator-based neutron source of the 7Li(p,n) reaction produced by 2.5 MeV protons was investigated by comparing the neutron beam tailored by both the Hiroshima University radiological research accelerator (HIRRAC) and the heavy water neutron irradiation facility in the Kyoto University reactor (KUR-HWNIF) from the viewpoint of the contamination dose ratios of the fast neutrons and the gamma rays. These contamination ratios to the boron dose were estimated in a water phantom of 20 cm diameter and 20 cm length to simulate a human head, with experiments by the same techniques for NCT in KUR-HWNIF and/or the simulation calculations by the Monte Carlo N-particle transport code system version 4B (MCNP-4B). It was found that the 7Li(p,n) neutrons produced by 2.5 MeV protons combined with 20, 25 or 30 cm thick D20 moderators of 20 cm diameter could make irradiation fields for NCT with depth-dose characteristics similar to those from the epithermal neutron beam at the KUR-HWNIF.

  9. Lithium ion dynamics in Li2S+GeS2+GeO2 glasses studied using (7)Li NMR field-cycling relaxometry and line-shape analysis.

    PubMed

    Gabriel, Jan; Petrov, Oleg V; Kim, Youngsik; Martin, Steve W; Vogel, Michael

    2015-09-01

    We use (7)Li NMR to study the ionic jump motion in ternary 0.5Li2S+0.5[(1-x)GeS2+xGeO2] glassy lithium ion conductors. Exploring the "mixed glass former effect" in this system led to the assumption of a homogeneous and random variation of diffusion barriers in this system. We exploit that combining traditional line-shape analysis with novel field-cycling relaxometry, it is possible to measure the spectral density of the ionic jump motion in broad frequency and temperature ranges and, thus, to determine the distribution of activation energies. Two models are employed to parameterize the (7)Li NMR data, namely, the multi-exponential autocorrelation function model and the power-law waiting times model. Careful evaluation of both of these models indicates a broadly inhomogeneous energy landscape for both the single (x=0.0) and the mixed (x=0.1) network former glasses. The multi-exponential autocorrelation function model can be well described by a Gaussian distribution of activation barriers. Applicability of the methods used and their sensitivity to microscopic details of ionic motion are discussed.

  10. Irradiation of nuclear track emulsions with thermal neutrons, heavy ions, and muons

    SciTech Connect

    Artemenkov, D. A. Bradnova, V.; Zaitsev, A. A.; Zarubin, P. I.; Zarubina, I. G.; Kattabekov, R. R.; Mamatkulov, K. Z.; Rusakova, V. V.

    2015-07-15

    Exposures of test samples of nuclear track emulsion were analyzed. Angular and energy correlations of products originating from the thermal-neutron-induced reaction n{sub th} +{sup 10} B → {sup 7} Li + (γ)+ α were studied in nuclear track emulsions enriched in boron. Nuclear track emulsions were also irradiated with {sup 86}Kr{sup +17} and {sup 124}Xe{sup +26} ions of energy about 1.2 MeV per nucleon. Measurements of ranges of heavy ions in nuclear track emulsionsmade it possible to determine their energies on the basis of the SRIM model. The formation of high-multiplicity nuclear stars was observed upon irradiating nuclear track emulsions with ultrarelativistic muons. Kinematical features studied in this exposure of nuclear track emulsions for events of the muon-induced splitting of carbon nuclei to three alpha particles are indicative of the nucleardiffraction interaction mechanism.

  11. Indirect measurement of nuclear reactions of astrophysical interest

    SciTech Connect

    Liu, W. P.; Li, Z. H.; Bai, X. X.; Wang, Y. B.; Guo, B.; Lian, G.; Su, J.; Zeng, S.; Wang, B. X.; Yan, S. Q.; Li, Y. J.; Li, E. T.; Jin, S. J.

    2010-05-12

    Systematic indirect measurements of nuclear astrophysical reactions using the unstable ion beam facility GIRAFFE in CIAE were performed. We have measured the angular distributions of transfer reactions, such as {sup 8}Li(d,p){sup 9}Li, {sup 8}Li(d,n){sup 9}Be and {sup 8}Li(p,d){sup 7}Li in inverse kinematics, and derived the astrophysical S-factors or reaction rates for {sup 8}Li(n,gamma){sup 9}Li and {sup 8}Li(p,gamma){sup 9}Be by using asymptotic normalization coefficient (ANC) or spectroscopic factor methods.

  12. Search for rare nuclear decays with HPGe detectors at the STELLA facility of the LNGS

    SciTech Connect

    Belli, P.; Di Marco, A.; Bernabei, R.; D'Angelo, S.; Cappella, F.; D'Angelo, A.; Incicchitti, A.; Cerulli, R.; Di Vacri, M. L.; Laubenstein, M.; Nisi, S.; Danevich, F. A.; Kobychev, V. V.; Poda, D. V.; Tretyak, V. I.; Kovtun, G. P.; Kovtun, N. G.; Shcherban, A. P.; Solopikhin, D. A.; Polischuk, O. G.; and others

    2013-12-30

    Results on the search for rare nuclear decays with the ultra low background facility STELLA at the LNGS using gamma ray spectrometry are presented. In particular, the best T{sub 1/2} limits were obtained for double beta processes in {sup 96}Ru and {sup 104}Ru. Several isotopes, which potentially decay through different 2β channels, including also possible resonant double electron captures, were investigated for the first time ({sup 156}Dy, {sup 158}Dy, {sup 184}Os, {sup 192}Os, {sup 190}Pt, {sup 198}Pt). Search for resonant absorption of solar {sup 7}Li axions in a LiF crystal gave the best limit for the mass of {sup 7}Li axions (< 8.6 keV). Rare alpha decay of {sup 190}Pt to the first excited level of {sup 186}Os(E{sub exc} = 137.2keV) was observed for the first time.

  13. Stopping powers of sup 7 Li, sup 11 B, sup 12 C, sup 14 N, and sup 16 O ions in C sub 16 H sub 14 O sub 3 polycarbonate

    SciTech Connect

    Rauhala, E.; Raeisaenen, J. )

    1990-09-01

    The stopping powers of bisphenol {ital A}-polycarbonate C{sub 16}H{sub 14}O{sub 3} for {sup 7}Li, {sup 11}B, {sup 12}C, {sup 14}N, and {sup 16}O ions in the 0.5--2.1-MeV/amu energy region have been determined. To avoid direct beam exposure on the film, a modified transmission geometry was used. The areal density of the foil, at exactly the position where the stopping power data were measured, was obtained by combining weighing and proton energy-loss measurements. The experimental stopping powers are compared with predictions of three semiempirical models, which are based on the heavy-ion scaling rule, and with our previous data for the same ions in Mylar. The systematics and deviations of the data from the predicted stopping powers, and the validity of Bragg's additivity rule, are discussed.

  14. Lithium Ion Mobility in Lithium Phosphidosilicates: Crystal Structure, (7) Li, (29) Si, and (31) P MAS NMR Spectroscopy, and Impedance Spectroscopy of Li8 SiP4 and Li2 SiP2.

    PubMed

    Toffoletti, Lorenzo; Kirchhain, Holger; Landesfeind, Johannes; Klein, Wilhelm; van Wüllen, Leo; Gasteiger, Hubert A; Fässler, Thomas F

    2016-12-05

    The need to improve electrodes and Li-ion conducting materials for rechargeable all-solid-state batteries has drawn enhanced attention to the investigation of lithium-rich compounds. The study of the ternary system Li-Si-P revealed a series of new compounds, two of which, Li8 SiP4 and Li2 SiP2 , are presented. Both phases represent members of a new family of Li ion conductors that display Li ion conductivity in the range from 1.15(7)×10(-6) Scm(-1) at 0 °C to 1.2(2)×10(-4) Scm(-1) at 75 °C (Li8 SiP4 ) and from 6.1(7)×10(-8) Scm(-1) at 0 °C to 6(1)×10(-6) Scm(-1) at 75 °C (Li2 SiP2 ), as determined by impedance measurements. Temperature-dependent solid-state (7) Li NMR spectroscopy revealed low activation energies of about 36 kJ mol(-1) for Li8 SiP4 and about 47 kJ mol(-1) for Li2 SiP2 . Both compounds were structurally characterized by X-ray diffraction analysis (single crystal and powder methods) and by (7) Li, (29) Si, and (31) P MAS NMR spectroscopy. Both phases consist of tetrahedral SiP4 anions and Li counterions. Li8 SiP4 contains isolated SiP4 units surrounded by Li atoms, while Li2 SiP2 comprises a three-dimensional network based on corner-sharing SiP4 tetrahedra, with the Li ions located in cavities and channels. © 2016 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

  15. Nuclear-spin-independent short-range three-body physics in ultracold atoms.

    PubMed

    Gross, Noam; Shotan, Zav; Kokkelmans, Servaas; Khaykovich, Lev

    2010-09-03

    We investigate three-body recombination loss across a Feshbach resonance in a gas of ultracold 7Li atoms prepared in the absolute ground state and perform a comparison with previously reported results of a different nuclear-spin state [N. Gross, Phys. Rev. Lett. 103, 163202 (2009)]. We extend the previously reported universality in three-body recombination loss across a Feshbach resonance to the absolute ground state. We show that the positions and widths of recombination minima and Efimov resonances are identical for both states which indicates that the short-range physics is nuclear-spin independent.

  16. Lithium glass scintillator neutron detector as an improved alternative to the standard 3 he proportional counter

    SciTech Connect

    Vladimir Popov, Pavel Degtiarenko

    2011-06-01

    Lithium glass scintillator made from 6Li-enriched substrate is a well known for its neutron detection capability. In spite of neutron interaction, cross section of 6Li happens to be lower than that of 3He. However, the neutron detection efficiency could be higher due to higher volume content of 6Li nuclear in the solid scintillator vs. gas filled proportional counter. At the same time, as lithium glass is sensitive to gamma and charge particle radiation, non-neutron radiation discrimination is required. Our detector is composed of two equal-size cylindrical Li(Ce) glass scintillators. The first one is high-sensitive to thermal neutrons GS-20 (6Li doped), the second one is GS-30 (7Li doped) type Scint-Gobain made lithium glass scintillator. Each of scintillators is coupled with R7400U Hamamatsu subminiature photomultiplier tube, and all assembly is fitted into NP100H 3He tube size. 6Li absorbs thermal neutrons releasing alpha particles and triton with 4.8 MeV total energy deposit inside the scintillator (equivalent to about ~1.3 MeV gamma energy depositions). Because 7Li isotope does not absorb thermal neutrons, and the physical properties of the two scintillators are virtually identical, the difference between these two scintillators could be used to provide neutron dose rate information. Results of study of neutron detector assembled of two Li(Ce) scintillators and NP100H moderator are presented

  17. Isotopic evidence ( 87Sr/ 86Sr, δ 7Li) for alteration of the oceanic crust at deep-rooted mud volcanoes in the Gulf of Cadiz, NE Atlantic Ocean

    NASA Astrophysics Data System (ADS)

    Scholz, Florian; Hensen, Christian; Reitz, Anja; Romer, Rolf L.; Liebetrau, Volker; Meixner, Anette; Weise, Stephan M.; Haeckel, Matthias

    2009-09-01

    The chemical and isotopic composition of pore fluids is presented for five deep-rooted mud volcanoes aligned on a transect across the Gulf of Cadiz continental margin at water depths between 350 and 3860 m. Generally decreasing interstitial Li concentrations and 87Sr/ 86Sr ratios with increasing distance from shore are attributed to systematically changing fluid sources across the continental margin. Although highest Li concentrations at the near-shore mud volcanoes coincide with high salinities derived from dissolution of halite and late-stage evaporites, clayey, terrigenous sediments are identified as the ultimate Li source to all pore fluids investigated. Light δ 7Li values, partly close to those of hydrothermal vent fluids (δ 7Li: +11.9‰), indicate that Li has been mobilized during high-temperature fluid/sediment or fluid/rock interactions in the deep sub-surface. Intense leaching of terrigenous clay has led to radiogenic 87Sr/ 86Sr ratios (˜0.7106) in pore fluids of the near-shore mud volcanoes. In contrast, non-radiogenic 87Sr/ 86Sr ratios (˜0.7075) at the distal locations are attributed to admixing of a basement-derived fluid component, carrying an isotopic signature from interaction with the basaltic crust. This inference is substantiated by temperature constraints from Li isotope equilibrium calculations suggesting exchange processes at particularly high temperatures (>200 °C) for the least radiogenic pore fluids of the most distal location. Advective pore fluids in the off-shore reaches of the Gulf of Cadiz are influenced by successive exchange processes with both oceanic crust and terrigenous, fine-grained sediments, resulting in a chemical and isotopic signature similar to that of fluids in near-shore ridge flank hydrothermal systems. This suggests that deep-rooted mud volcanoes in the Gulf of Cadiz represent a fluid pathway intermediate between mid-ocean ridge hydrothermal vent and shallow, marginal cold seep. Due to the thicker sediment

  18. Synthesis, crystal chemistry, and magnetic properties of RE7Li8Ge10 and RE11Li12Ge16 (RE = La-Nd, Sm): new members of the [REGe2](n)[RELi2Ge](m) homologous series.

    PubMed

    Guo, Sheng-Ping; You, Tae-Soo; Jung, Ya-Ho; Bobev, Svilen

    2012-06-18

    Eight new rare-earth metal-lithium-germanides belonging to the [REGe(2)](n)[RELi(2)Ge](m) homologous series have been synthesized and structurally characterized by single-crystal X-ray diffraction. The structures of the title compounds can be rationalized as linear intergrowths of imaginary RELi(2)Ge (MgAl(2)Cu structure type) and REGe(2) (AlB(2) structure type) slabs. The compounds with general formula RE(7)Li(8)Ge(10) (RE = La-Nd, Sm), i.e., [REGe(2)](3)[RELi(2)Ge](4), crystallize in the orthorhombic space group Cmmm (No. 65) with a new structure type. Similarly, the compounds with general formula RE(11)Li(12)Ge(16) (RE = Ce-Nd), i.e., [REGe(2)](5)[RELi(2)Ge](6), crystallize in the orthorhombic space group Immm (No. 71) also with its own structure type. Temperature-dependent DC magnetization measurements indicate Curie-Weiss paramagnetism in the high-temperature regime and hint at complex magnetic ordering at low temperatures. The measured effective moments are consistent with RE(3+) ground states in all cases. The experimental results have been complemented by tight-binding linear muffin-tin orbital (TB-LMTO) electronic structure calculations.

  19. Production of 93mMo through natY(7Li, 3n) reaction and subsequent studies on separation and extraction behaviour of no-carrier-added 93mMo from an yttrium target.

    PubMed

    Nayak, Dalia; Lahiri, Susanta

    2008-12-01

    The present work reports heavy-ion-assisted production of (93m)Mo from a natural yttrium target using the (89)Y((7)Li, 3n)(93m)Mo reaction. Three different methodologies based on liquid-liquid extraction (LLX), aqueous biphasic extraction and precipitation, have been developed for separation and extraction of no-carrier-added (nca) (93m)Mo (T(1/2)=6.85h) radionuclide from bulk yttrium target. Complete separation of nca Mo from the target Y has been achieved by employing LLX technique with 0.1M trioctylamine (TOA) dissolved in cyclohexane and 8M HCl. Quantitative separation of (93m)Mo from the yttrium target is also possible by precipitating bulk yttrium with 1M oxalic acid. However, for this particular case, studies have shown that the aqueous biphasic extraction is not the method of choice for separation of nca Mo. Nevertheless, the extraction pattern is important in the context of simulation experiments for studying the behaviour of (106)Sg. Similarity or dissimilarity between the extraction patterns in various analytical systems will be helpful to decisively place Sg in the right position in the periodic table.

  20. Physical and electrochemical characterization of 0.3Li2MnO3 x 0.7LiMn0.60Ni0.25Co0.15O2 material for Li secondary battery.

    PubMed

    Kim, Jeong-Min; Choi, Man-Soo; Jin, Bong-Soo; Wang, Guoxiu; Kim, Hyun-Soo

    2014-10-01

    The 0.3Li2MnO3 x 0.7LiMn0.60Ni0.25Co0.15O2 cathode materials were synthesized using a coprecipitation method at a various heat-treatment temperature. From XRD pattern analysis, pure layered structure without impurities was confirmed from all samples and the peak intensity of Li2MnO3 was increased as the heat-treatment temperature increased. The primary particle size increased approximately from 100 nm to 500 nm with increasing heat-treatment temperature. The initial discharge capacity of the materials obtained at 950 degrees C was 235 mA h/g at 0.1 C rate, but then decreased down to 228 mA h/g with further increasing heat-treatment temperature. And, in the voltage range of 2.0-4.6 V, the electrode heat-treated at 900 degrees C showed the highest capacity retention of 68% at 5 C rate against to 0.1 C rate.

  1. NMR spin-lattice relaxation study of {sup 7}Li and {sup 93}Nb nuclei in Ti- or Fe-doped LiNbO{sub 3}:Mg single crystals

    SciTech Connect

    Yeom, Tae Ho; Lim, Ae Ran E-mail: arlim@jj.ac.kr

    2016-04-15

    In this study, to understand the effects of paramagnetic impurities, we investigated the temperature dependent of the spin-lattice relaxation times of pure LiNbO{sub 3}, LiNbO{sub 3}:Mg, LiNbO{sub 3}:Mg/Ti, LiNbO{sub 3}:Mg/Fe, and LiNbO{sub 3}:Mg/Fe (thermally treated at 500°C) single crystals. The results for the LiNbO{sub 3}:Mg single crystals doped with Fe{sup 3+} or Ti{sup 3+} are discussed with respect to the site distribution and atomic mobility of Li and Nb. In addition, the effects of a thermal treatment on LiNbO{sub 3}:Mg/Fe single crystals were examined based on the T{sub 1} analysis of {sup 7}Li and {sup 93}Nb. It was found that the presence of impurities in the crystals induced systematic changes of activation energies concerning atomic mobility.

  2. Laser inertial fusion-based energy: Neutronic design aspects of a hybrid fusion-fission nuclear energy system

    NASA Astrophysics Data System (ADS)

    Kramer, Kevin James

    the same radial flibe flow that travels through perforated ODS walls to the reflector blanket. This reflector blanket is 75 cm thick comprised of 2 cm diameter graphite pebbles cooled by flibe. The flibe extraction plenum surrounds the reflector bed. Detailed neutronics designs studies are performed to arrive at the described design. The LFFH engine thermal power is controlled using a technique of adjusting the 6Li/7Li enrichment in the primary and secondary coolants. The enrichment adjusts system thermal power in the design by increasing tritium production while reducing fission. To perform the simulations and design of the LFFH engine, a new software program named LFFH Nuclear Control (LNC) was developed in C++ to extend the functionality of existing neutron transport and depletion software programs. Neutron transport calculations are performed with MCNP5. Depletion calculations are performed using Monteburns 2.0, which utilizes ORIGEN 2.0 and MCNP5 to perform a burnup calculation. LNC supports many design parameters and is capable of performing a full 3D system simulation from initial startup to full burnup. It is able to iteratively search for coolant 6Li enrichments and resulting material compositions that meet user defined performance criteria. LNC is utilized throughout this study for time dependent simulation of the LFFH engine. Two additional methods were developed to improve the computation efficiency of LNC calculations. These methods, termed adaptive time stepping and adaptive mesh refinement were incorporated into a separate stand alone C++ library name the Adaptive Burnup Library (ABL). The ABL allows for other client codes to call and utilize its functionality. Adaptive time stepping is useful for automatically maximizing the size of the depletion time step while maintaining a desired level of accuracy. Adaptive meshing allows for analysis of fixed fuel configurations that would normally require a computationally burdensome number of depletion zones

  3. Nuclear power and nuclear weapons

    SciTech Connect

    Vaughen, V.C.A.

    1983-01-01

    The proliferation of nuclear weapons and the expanded use of nuclear energy for the production of electricity and other peaceful uses are compared. The difference in technologies associated with nuclear weapons and nuclear power plants are described.

  4. Nuclear rights - nuclear wrongs

    SciTech Connect

    Paul, E.F.; Miller, F.D.; Paul, J.; Ahrens, J.

    1986-01-01

    This book contains 11 selections. The titles are: Three Ways to Kill Innocent Bystanders: Some Conundrums Concerning the Morality of War; The International Defense of Liberty; Two Concepts of Deterrence; Nuclear Deterrence and Arms Control; Ethical Issues for the 1980s; The Moral Status of Nuclear Deterrent Threats; Optimal Deterrence; Morality and Paradoxical Deterrence; Immoral Risks: A Deontological Critique of Nuclear Deterrence; No War Without Dictatorship, No Peace Without Democracy: Foreign Policy as Domestic Politics; Marxism-Leninism and its Strategic Implications for the United States; Tocqueveille War.

  5. Excitation functions and isomer ratio measurements for the reaction /sup 41/K(/sup 6/Li,p2n)/sup 44/Sc/sup m/,/sup 44/Sc/sup q/. [14. 4, 23. 4, 32. 0, and 41. 5 MeV

    SciTech Connect

    Nguyen, H.D.; Trinh, H.N.; Le, H.D.; Moody, K.J.; Groening, H.; Seaborg, G.T.

    1981-10-01

    For the purpose of eventually determining how population distributions of /sup 44/Sc* in the E-J plane affect resulting isomer ratios in /sup 44/Sc, excitation functions and isomer ratios in the reaction /sup 41/K(/sup 6/Li,p2n)/sup 44/Sc/sup m/,/sup 44/Sc/sup q/ were measured. Preliminary results seem to indicate, as expected, a very weak compound nucleus reaction component of the reaction cross section.

  6. Refined scenario of standard Big Bang nucleosynthesis allowing for nonthermal nuclear reactions in the primordial plasma

    SciTech Connect

    Voronchev, Victor T.; Nakao, Yasuyuki; Nakamura, Makoto; Tsukida, Kazuki

    2012-11-12

    The standard scenario of big bang nucleosynthesis (BBN) is generalized to take into account nonthermal nuclear reactions in the primordial plasma. These reactions are naturally triggered in the BBN epoch by fast particles generated in various exoergic processes. It is found that, although such particles can appreciably enhance the rates of some individual reactions, their influence on the whole process of element production is not significant. The nonthermal corrections to element abundances are obtained to be 0.1% ({sup 3}H), -0.03% ({sup 7}Li), and 0.34 %-0.63% (CNO group).

  7. Characterization of moderator assembly dimension for accelerator boron neutron capture therapy of brain tumors using 7Li(p, n) neutrons at proton energy of 2.5 MeV.

    PubMed

    Tanaka, Kenichi; Kobayashi, Tooru; Bengua, Gerard; Nakagawa, Yoshinobu; Endo, Satoru; Hoshi, Masaharu

    2006-06-01

    The characteristics of moderator assembly dimension are investigated for the usage of 7Li(p,n) neutrons by 2.5 MeV protons in boron newtron capture therapy (BNCT) of brain tumors in the present study. The indexes checked are treatable protocol depth (TPD), which is the greatest depth of the region satisfying the dose requirements in BNCT protocol, proton current necessary to complete BNCT by 1 h irradiation, and the heat flux deposited in the Li target which should be removed. Assumed materials are D2O for moderator, and mixture of polyethylene and LiF with 50 wt % for collimator. Dose distributions have been computed with MCNP 4B and 4C codes. Consequently, realized TPD does not show a monotonical tendency for the Li target diameter. However, the necessary proton current and heat flux in the Li target decreases as the Li target diameter increases, while this trend reverses at around 10 cm of the Li target diameter for the necessary proton current in the condition of this study. As to the moderator diameter, TPD does not exhibit an apparent dependence. On the other hand, necessary proton current and heat flux decrease as the moderator diameter increases, and this tendency saturates at around 60 cm of the moderator diameter in this study. As to the collimator, increase in inner diameter is suitable from the viewpoint of increasing TPD and decreasing necessary proton current and heat flux, while these indexes do not show apparent difference for collimator inner diameters over 14 cm for the parameters treated here. The practical viewpoint in selecting the parameters of moderator assembly dimension is to increase TPD, within the technically possible condition of accelerated proton current and heat removal from the Li target. In this process, the values for which the resultant characteristics mentioned above saturate or reverse would be important factors.

  8. Characterization of moderator assembly dimension for accelerator boron neutron capture therapy of brain tumors using {sup 7}Li(p,n) neutrons at proton energy of 2.5 MeV

    SciTech Connect

    Tanaka, Kenichi; Kobayashi, Tooru; Bengua, Gerard; Nakagawa, Yoshinobu; Endo, Satoru; Hoshi, Masaharu

    2006-06-15

    The characteristics of moderator assembly dimension are investigated for the usage of {sup 7}Li(p,n) neutrons by 2.5 MeV protons in boron newtron capture therapy (BNCT) of brain tumors in the present study. The indexes checked are treatable protocol depth (TPD), which is the greatest depth of the region satisfying the dose requirements in BNCT protocol, proton current necessary to complete BNCT by 1 h irradiation, and the heat flux deposited in the Li target which should be removed. Assumed materials are D{sub 2}O for moderator, and mixture of polyethylene and LiF with 50 wt % for collimator. Dose distributions have been computed with MCNP 4B and 4C codes. Consequently, realized TPD does not show a monotonical tendency for the Li target diameter. However, the necessary proton current and heat flux in the Li target decreases as the Li target diameter increases, while this trend reverses at around 10 cm of the Li target diameter for the necessary proton current in the condition of this study. As to the moderator diameter, TPD does not exhibit an apparent dependence. On the other hand, necessary proton current and heat flux decrease as the moderator diameter increases, and this tendency saturates at around 60 cm of the moderator diameter in this study. As to the collimator, increase in inner diameter is suitable from the viewpoint of increasing TPD and decreasing necessary proton current and heat flux, while these indexes do not show apparent difference for collimator inner diameters over 14 cm for the parameters treated here. The practical viewpoint in selecting the parameters of moderator assembly dimension is to increase TPD, within the technically possible condition of accelerated proton current and heat removal from the Li target. In this process, the values for which the resultant characteristics mentioned above saturate or reverse would be important factors.

  9. PRODUCTION OF {sup 9}Be THROUGH THE {alpha}-FUSION REACTION OF METAL-POOR COSMIC RAYS AND STELLAR FLARES

    SciTech Connect

    Kusakabe, Motohiko; Kawasaki, Masahiro E-mail: kawasaki@icrr.u-tokyo.ac.jp

    2013-04-10

    Spectroscopic observations of metal-poor stars have indicated possible {sup 6}Li abundances that are much larger than the primordial abundance predicted in the standard big bang nucleosynthesis model. Possible mechanisms of {sup 6}Li production in metal-poor stars include pregalactic and cosmological cosmic-ray (CR) nucleosynthesis and nucleosynthesis by flare-accelerated nuclides. We study {sup 9}Be production via two-step {alpha}-fusion reactions of CR or flare-accelerated {sup 3,4}He through {sup 6}He and {sup 6,7}Li, in pregalactic structure, intergalactic medium, and stellar surfaces. We solve transfer equations of CR or flare particles and calculate nuclear yields of {sup 6}He, {sup 6,7}Li, and {sup 9}Be taking account of probabilities of processing {sup 6}He and {sup 6,7}Li into {sup 9}Be via fusions with {alpha} particles. Yield ratios, i.e., {sup 9}Be/{sup 6}Li, are then calculated for the CR and flare nucleosynthesis models. We suggest that the future observations of {sup 9}Be in metal-poor stars may find enhanced abundances originating from metal-poor CR or flare activities.

  10. Nuclear Medicine.

    ERIC Educational Resources Information Center

    Badawi, Ramsey D.

    2001-01-01

    Describes the use of nuclear medicine techniques in diagnosis and therapy. Describes instrumentation in diagnostic nuclear medicine and predicts future trends in nuclear medicine imaging technology. (Author/MM)

  11. Nuclear ventriculography

    MedlinePlus

    ... ventriculography (RNV); Multiple gate acquisition scan (MUGA); Nuclear cardiology; Cardiomyopathy - nuclear ventriculography ... 56. Udelson JE, Dilsizian V, Bonow RO. Nuclear cardiology. In: Bonow RO, Mann DL, Zipes DP, Libby ...

  12. Nuclear Medicine.

    ERIC Educational Resources Information Center

    Badawi, Ramsey D.

    2001-01-01

    Describes the use of nuclear medicine techniques in diagnosis and therapy. Describes instrumentation in diagnostic nuclear medicine and predicts future trends in nuclear medicine imaging technology. (Author/MM)

  13. Nuclear data for nuclear transmutation

    SciTech Connect

    Harada, Hideo

    2009-05-04

    Current status on nuclear data for the study of nuclear transmutation of radioactive wastes is reviewed, mainly focusing on neutron capture reactions. It is stressed that the highest-precision frontier research in nuclear data measurements should be a key to satisfy the target accuracies on the nuclear data requested for realizing the nuclear transmutation.

  14. Nuclear data for nuclear transmutation

    NASA Astrophysics Data System (ADS)

    Harada, Hideo

    2009-05-01

    Current status on nuclear data for the study of nuclear transmutation of radioactive wastes is reviewed, mainly focusing on neutron capture reactions. It is stressed that the highest-precision frontier research in nuclear data measurements should be a key to satisfy the target accuracies on the nuclear data requested for realizing the nuclear transmutation.

  15. Theory of the Lamb shift in muonic ions μ Li, μ Be, μ B

    NASA Astrophysics Data System (ADS)

    Krutov, A. A.; Martynenko, A. P.; Martynenko, F. A.; Sukhorukova, O. S.

    2017-09-01

    The calculation of the Lamb shift 2 P 1/2 - 2 S 1/2 in muonic ions (μ 3 6 Li)2+, (μ 3 7 Li)2+, (μ 4 9 Be)3+, (μ 4 10 Be)3+, (μ 5 10 B)4+, (μ 5 11 B)4+, is performed taking into account the corrections of order α3, α4, α5, α6 to the vacuum polarization, nuclear structure and recoil. The dependence of numerical values of the contributions from the nuclear charge is carried out. The obtained results can be used for extracting more accurate values of nuclear charge radii of nuclei of future experiments.

  16. Passive sensor systems for nuclear material monitoring

    SciTech Connect

    Simpson, M.L.; Boatner, L.A.; Holcomb, D.E.; McElhaney, S.A.; Mihalczo, J.T.; Muhs, J.D.; Roberts, M.R.; Hill, N.W.

    1993-09-01

    Passive fiber optic sensor systems capable of confirming the presence of special nuclear materials in storage or process facilities are being developed at Oak Ridge National Laboratory (ORNL). These sensors provide completely passive, remote measurement capability. No power supplies, amplifiers, or other active components that could degrade system reliability are required at the sensor location. ORNL, through its research programs in scintillator materials, has developed a variety of materials for use in alpha-, beta-, gamma-, and neutron-sensitive scintillator detectors. In addition to sensors for measuring radiation flux, new sensor materials have been developed which are capable of measuring weight, temperature, and source location. An example of a passive sensor for temperature measurement is the combination of a thermophosphor (e.g., rare-earth activated Y{sub 2}O{sub 3}) with {sup 6}LiF (95% {sup 6}Li). This combination results in a new class of scintillators for thermal neutrons that absorb energy from the radiation particles and remit the energy as a light pulse, the decay rate of which, over a specified temperature range, is temperature dependent. Other passive sensors being developed include pressure-sensitive triboluminescent materials, weight-sensitive silicone rubber fibers, scintillating fibers, and other materials for gamma and neutron detection. The light from the scintillator materials of each sensor would be sent through optical fibers to a monitoring station, where the attribute quantity could be measured and compared with previously recorded emission levels. Confirmatory measurement applications of these technologies are being evaluated to reduce the effort, costs, and employee exposures associated with inventorying stockpiles of highly enriched uranium at the Oak Ridge Y-12 Plant.

  17. Colorado School of Mines low energy nuclear physics project

    SciTech Connect

    Cecil, F.E.

    1991-01-02

    A major accomplishment of this project in the past year is the completion of a fairly comprehensive paper describing the survey of radiative capture reactions of protons on light nuclei at low energies. In addition we have completed a preliminary set of measurements of (d,p)/(d,{alpha}) cross section ratios on the charge symmetric nuclei {sup 6}Li and {sup 10}B as a test of the Oppenheimer-Phillips effect. While the {sup 6}Li data remain inconclusive, the {sup 10}B data show solid evidence for the Oppenheimer-Phillips enhancement of the (d,p) reaction relative to the (d,{alpha}) reaction for deuteron bombarding energies below about 100 keV. We have continued our investigation of fusion reaction products from deuterium-metal systems at room temperatures with the startling observation of intense burst of energetic charged particles from deuterium gas loaded thin titaium foils subject to non-equilibrium thermal and electrical conditions. We have completed two projects involving the application of the low energy particle accelerator to material science problems; firstly a study of the transformation of crystalline to amorphous Fe-Zr systems by proton irradiation and secondly the effects of ion bombardment on the critical temperature of YBCO high-temperature superconductors. Finally we have made progress in several instrumentation projects which will be used in some of the up-coming measurements of nuclear cross sections at very low energies.

  18. Trojan horse particle invariance: The impact on nuclear astrophysics

    NASA Astrophysics Data System (ADS)

    Pizzone, R. G.; Spitaleri, C.; Bertulani, C. A.; Mukhamedzhanov, A. M.; Blokhintsev, L. D.; La Cognata, M.; Lamia, L.; Spartá, R.; Tumino, A.

    2014-05-01

    In the current picture of nuclear astrophysics indirect methods and, in particular, the Trojan Horse Method cover a crucial role for the measurement of charged particle induced reactions cross sections of astrophysical interest, in the energy range required by the astrophysical scenarios. To better understand its cornerstones and its applications to physical cases many tests were performed to verify all its properties and the possible future perspectives. The key to the method is the quasi-free break-up and some of its properties will be investigated in the present work. In particular, the Trojan Horse nucleus invariance will be studied and previous studies will be extended to the cases of the binary d(d, p)t and 6Li(d,α)4He reactions, which were tested using different quasi-free break-up's, namely 6Li and 3He. The astrophysical S(E)-factor were then extracted with the Trojan Horse formalism applied to the two different break-up schemes and compared with direct data as well as with previous indirect investigations. The very good agreement confirms the independence of binary indirect cross section on the chosen spectator particle also for these reactions.

  19. Trojan horse particle invariance: The impact on nuclear astrophysics

    SciTech Connect

    Pizzone, R. G.; La Cognata, M.; Spitaleri, C.; Bertulani, C. A.; Mukhamedzhanov, A. M.; Blokhintsev, L. D.; Lamia, L.; Spartá, R.; Tumino, A.

    2014-05-02

    In the current picture of nuclear astrophysics indirect methods and, in particular, the Trojan Horse Method cover a crucial role for the measurement of charged particle induced reactions cross sections of astrophysical interest, in the energy range required by the astrophysical scenarios. To better understand its cornerstones and its applications to physical cases many tests were performed to verify all its properties and the possible future perspectives. The key to the method is the quasi-free break-up and some of its properties will be investigated in the present work. In particular, the Trojan Horse nucleus invariance will be studied and previous studies will be extended to the cases of the binary d(d, p)t and {sup 6}Li(d,α){sup 4}He reactions, which were tested using different quasi-free break-up's, namely {sup 6}Li and {sup 3}He. The astrophysical S(E)-factor were then extracted with the Trojan Horse formalism applied to the two different break-up schemes and compared with direct data as well as with previous indirect investigations. The very good agreement confirms the independence of binary indirect cross section on the chosen spectator particle also for these reactions.

  20. Coulomb and nuclear effects in breakup and reaction cross sections

    NASA Astrophysics Data System (ADS)

    Descouvemont, P.; Canto, L. F.; Hussein, M. S.

    2017-01-01

    We use a three-body continuum discretized coupled channel (CDCC) model to investigate Coulomb and nuclear effects in breakup and reaction cross sections. The breakup of the projectile is simulated by a finite number of square integrable wave functions. First we show that the scattering matrices can be split in a nuclear term and in a Coulomb term. This decomposition is based on the Lippmann-Schwinger equation and requires the scattering wave functions. We present two different methods to separate both effects. Then, we apply this separation to breakup and reaction cross sections of 7Li+208Pb . For breakup, we investigate various aspects, such as the role of the α +t continuum, the angular-momentum distribution, and the balance between Coulomb and nuclear effects. We show that there is a large ambiguity in defining the Coulomb and nuclear breakup cross sections, since both techniques, although providing the same total breakup cross sections, strongly differ for the individual components. We suggest a third method which could be efficiently used to address convergence problems at large angular momentum. For reaction cross sections, interference effects are smaller, and the nuclear contribution is dominant above the Coulomb barrier. We also draw attention to different definitions of the reaction cross section which exist in the literature and which may induce small, but significant, differences in the numerical values.

  1. Nuclear Spectroscopy with HELIOS

    NASA Astrophysics Data System (ADS)

    Hoffman, Calem

    2013-04-01

    Direct reaction studies have been instrumental in achieving our current understanding of nuclear structure through the measurement of angular distributions, the extraction of spectroscopic factors, and the determination of single-particle centroids. Traditionally, these experiments were carried out using a beam of light particles impinging on a heavy stable target. Over the last decade this important technique has been used with short-lived radioactive ion beams requiring these types of reactions to be carried out in inverse kinematics. There are numerous challenges to this approach, not least is the typical Q-value resolution being up to an order of magnitude worse than traditional measurements due mainly to the so-called kinematic compression. The Helical Orbit Spectrometer (HELIOS) is a detection system developed for the specific purpose of improving the Q value resolution for inverse direct reaction measurements, while also maintaining flexibility and high efficiency. The novel feature of HELIOS is use of a 3 Tesla solenoid inside which the reactions take place. This allows for light particles of interest to be measured at fixed longitudinal distances from the target as opposed to fixed laboratory angles. The subtle mapping from laboratory angle to longitudinal position removes the aforementioned kinematic compression effect improving the Q-value resolution by as much as a factor of five without out sacrificing detection efficiency. In addition, HELIOS provides a natural way to identify particles of interest, independent of energy, through their measured cyclotron period. The design and implementation of HELIOS at the Argonne Tandem Linear Accelerator System (ATLAS) on the site of Argonne National Laboratory will be presented. The device has been extremely successful as numerous early measurements have been conducted spanning masses A=11 to 136, using varying reactions such as (d,p), (d,^3He), and (^6LI,d), as well as a range of beam energies. Physics

  2. Natural variations of lithium isotopes in a mammalian model.

    PubMed

    Balter, Vincent; Vigier, Nathalie

    2014-03-01

    Despite lithium's extensive clinical applications, the cellular and molecular basis for the therapeutic effects remains to be elucidated. The large difference in mass between the two lithium isotopes ((6)Li and (7)Li) has prompted biochemists to explore the metabolism of Li by using pure (6)Li and (7)Li labeled drugs. However, experiments were carried out at very high Li concentrations, which did not reflect natural conditions. In the present study, we consider, for the first time, the natural variations of the (7)Li/(6)Li ratio in the organs and body fluids of an animal model, sheep. Each organ seems to be characterized by a specific Li isotope composition. So far, the range of the (7)Li/(6)Li ratio in the sheep body, expressed as δ permil variations relative to the L-SVEC standard (δ(7)Li), is about 40‰, between muscles (∼40‰) and kidney (∼0‰). Relative to a dietary δ(7)Li value of ∼+17‰, serum, red blood cells, muscle, liver, brain and kidney have a (7)Li enrichment of -12‰, -14‰, +22‰, +5‰, -3‰ and -15‰, respectively. The Li isotope composition is likely to be fractionated during intestinal absorption, with a greater absorption of (6)Li relative to (7)Li. According to previous conclusions obtained with (6)Li and (7)Li labeled chemicals, (6)Li appears to diffuse into erythrocytes faster than does (7)Li. However, this does not hold for myocytes and hepatocytes, because these two tissues have a higher δ(7)Li level than serum. Purely diffusive isotopic fractionation would leave all organs (7)Li-depleted relative to the serum, which is not the case, suggesting that active, molecule-specific, isotopic fractionation occurs in the body. Our preliminary results suggest that natural Li isotope variations can shed light on its regulation in the body, being active or passive.

  3. Nuclear Chemistry.

    ERIC Educational Resources Information Center

    Chemical and Engineering News, 1979

    1979-01-01

    Provides a brief review of the latest developments in nuclear chemistry. Nuclear research today is directed toward increased activity in radiopharmaceuticals and formation of new isotopes by high-energy, heavy-ion collisions. (Author/BB)

  4. Nuclear Scans

    MedlinePlus

    Nuclear scans use radioactive substances to see structures and functions inside your body. They use a special ... images. Most scans take 20 to 45 minutes. Nuclear scans can help doctors diagnose many conditions, including ...

  5. Nuclear Winter.

    ERIC Educational Resources Information Center

    Ehrlich, Anne

    1984-01-01

    "Nuclear Winter" was recently coined to describe the climatic and biological effects of a nuclear war. These effects are discussed based on models, simulations, scenarios, and projections. Effects on human populations are also considered. (JN)

  6. Nuclear Medicine

    MedlinePlus

    ... Home » Science Education » Science Topics » Nuclear Medicine SCIENCE EDUCATION SCIENCE EDUCATION Science Topics Resource Links for General Public Resource ... Related Documents: Nuclear Medicine Fact Sheet.pdf SCIENCE EDUCATION Science Topics Resource Links for General Public Resource ...

  7. Nuclear Chemistry.

    ERIC Educational Resources Information Center

    Chemical and Engineering News, 1979

    1979-01-01

    Provides a brief review of the latest developments in nuclear chemistry. Nuclear research today is directed toward increased activity in radiopharmaceuticals and formation of new isotopes by high-energy, heavy-ion collisions. (Author/BB)

  8. Nuclear Winter.

    ERIC Educational Resources Information Center

    Ehrlich, Anne

    1984-01-01

    "Nuclear Winter" was recently coined to describe the climatic and biological effects of a nuclear war. These effects are discussed based on models, simulations, scenarios, and projections. Effects on human populations are also considered. (JN)

  9. Nuclear reaction uncertainties, massive gravitino decays and the cosmological lithium problem

    SciTech Connect

    Cyburt, Richard H.; Ellis, John; Fields, Brian D.; Luo, Feng; Olive, Keith A.; Spanos, Vassilis C. E-mail: john.ellis@cern.ch E-mail: fluo@physics.umn.edu E-mail: spanos@physics.umn.edu

    2010-10-01

    We consider the effects of uncertainties in nuclear reaction rates on the cosmological constraints on the decays of unstable particles during or after Big-Bang nucleosynthesis (BBN). We identify the nuclear reactions due to non-thermal hadrons that are the most important in perturbing standard BBN, then quantify the uncertainties in these reactions and in the resulting light-element abundances. These results also indicate the key nuclear processes for which improved cross section data would allow different light-element abundances to be determined more accurately, thereby making possible more precise probes of BBN and evaluations of the cosmological constraints on unstable particles. Applying this analysis to models with unstable gravitinos decaying into neutralinos, we calculate the likelihood function for the light-element abundances measured currently, taking into account the current experimental errors in the determinations of the relevant nuclear reaction rates. We find a region of the gravitino mass and abundance in which the abundances of deuterium, {sup 4}He and {sup 7}Li may be fit with χ{sup 2} = 5.5, compared with χ{sup 2} = 31.7 if the effects of gravitino decays are unimportant. The best-fit solution is improved to χ{sup 2} ∼ 2.0 when the lithium abundance is taken from globular cluster data. Some such re-evaluation of the observed light-element abundances and/or nuclear reaction rates would be needed if this region of gravitino parameters is to provide a complete solution to the cosmological {sup 7}Li problem.

  10. Nuclear weapons, nuclear effects, nuclear war

    SciTech Connect

    Bing, G.F.

    1991-08-20

    This paper provides a brief and mostly non-technical description of the militarily important features of nuclear weapons, of the physical phenomena associated with individual explosions, and of the expected or possible results of the use of many weapons in a nuclear war. Most emphasis is on the effects of so-called ``strategic exchanges.``

  11. Nuclear Fuels.

    ERIC Educational Resources Information Center

    Nash, J. Thomas

    1983-01-01

    Trends in and factors related to the nuclear industry and nuclear fuel production are discussed. Topics addressed include nuclear reactors, survival of the U.S. uranium industry, production costs, budget cuts by the Department of Energy and U.S. Geological survey for resource studies, mining, and research/development activities. (JN)

  12. Nuclear Fuels.

    ERIC Educational Resources Information Center

    Nash, J. Thomas

    1983-01-01

    Trends in and factors related to the nuclear industry and nuclear fuel production are discussed. Topics addressed include nuclear reactors, survival of the U.S. uranium industry, production costs, budget cuts by the Department of Energy and U.S. Geological survey for resource studies, mining, and research/development activities. (JN)

  13. New cold nuclear fusion theory and experimental tests

    NASA Astrophysics Data System (ADS)

    Kim, Yeong E.

    1990-12-01

    A theory of neutron-induced tritium-deuterium fusion at room temperature is developed, based entirely on previously measured cross-sections of known nuclear reactions. The fusion process involves self-sustaining chain reactions: (1) n+6Li →4He+T and/or n+7Li→4He+T+ n, and (2) T+D →4He+n, in Li-D plasma or pellet surrounded by Li and other blankets and by neutron reflectors. The recent results of cold deuterium fusion reported by Fleischmann, Pons, and Hawkins are described in terms of this fusion process. Experimental evidence and tests of the chain reaction hypothesis are described.

  14. Nuclear Pasta

    NASA Astrophysics Data System (ADS)

    da Silva Schneider, Andre; Horowitz, Charles; Berry, Don; Briggs, Christian

    2014-03-01

    For decades it has been theorized that just below nuclear saturation density matter undergoes a series of phase transitions. These phases, which are expected to exist in core-collapse supernovae and neutron stars, involve a range of exotic nuclear shapes collectively known as nuclear pasta. Recently, Jose Pons and collaborators suggested that ``the maximum period of isolated X-ray pulsars may be the first observational evidence for an amorphous inner crust, ..., possibly owing to the existence of a nuclear pasta phase.'' In this talk we present results of semi-classical molecular dynamics simulations of nuclear pasta and discuss how each phase might contribute to neutron star crust properties.

  15. Nuclear orientation and nuclear structure

    SciTech Connect

    Krane, K.S.

    1988-01-01

    The present generation of on-line nuclear orientation facilities promises to revolutionize the gathering of nuclear structure information, especially for the hitherto poorly known and understood nuclei far from stability. Following a brief review of the technological developments that have facilitated these experiments, the nuclear spectroscopic information that can be obtained is summarized. Applications to understanding nuclear structure are reviewed, and challenges for future studies are discussed. 14 refs., 4 figs., 3 tabs.

  16. Nuclear networking.

    PubMed

    Xie, Wei; Burke, Brian

    2017-07-04

    Nuclear lamins are intermediate filament proteins that represent important structural components of metazoan nuclear envelopes (NEs). By combining proteomics and superresolution microscopy, we recently reported that both A- and B-type nuclear lamins form spatially distinct filament networks at the nuclear periphery of mouse fibroblasts. In particular, A-type lamins exhibit differential association with nuclear pore complexes (NPCs). Our studies reveal that the nuclear lamina network in mammalian somatic cells is less ordered and more complex than that of amphibian oocytes, the only other system in which the lamina has been visualized at high resolution. In addition, the NPC component Tpr likely links NPCs to the A-type lamin network, an association that appears to be regulated by C-terminal modification of various A-type lamin isoforms. Many questions remain, however, concerning the structure and assembly of lamin filaments, as well as with their mode of association with other nuclear components such as peripheral chromatin.

  17. Decomposition of nuclear response functions for neutrino-induced reactions on 12C

    NASA Astrophysics Data System (ADS)

    Kim, Byungjick; Kim, K. S.; Kim, Hungchong; So, W. Y.; Cheoun, Myung-Ki

    2014-10-01

    We investigate the nuclear response functions in neutrino-induced reaction via a neutral current (NC) on 12C, which functions are comprised of Coulomb, longitudinal, magnetic and electric transitions. Those response functions in the NC reaction are closely related to those extracted from other types of NC reactions by electrons, protons and other light nuclei, such as A( e, e')A *, A( p, p')A *, A( d, d')A *, and A(6Li,6Li')A *. For example, the magnetic response function for the J π = 1+ state (M1) which is associated with the spin transfer reaction can be measured in inelastic scattering and may give us valuable information for the NC neutrino-induced reaction. Therefore, if we exploit response functions deduced by using other nuclear reactions, neutrino reactions could be estimated indirectly without relying on neutrino-induced reaction experiments. For the purpose, in this work, we decompose every response function in the neutrino reaction 12C( ν e , ν' e )12C*( J π = 1+) and address the role of each response function in the reaction.

  18. Tritium speciation in nuclear reactor bioshield concrete and its impact on accurate analysis.

    PubMed

    Kim, Dae Ji; E Warwick, Phillip; Croudace, Ian W

    2008-07-15

    Tritium ((3)H) is produced in nuclear reactors via several neutron-induced reactions [(2)H(n, gamma)(3)H, (6)Li(n, alpha)(3)H, (10)B(n, 2alpha)(3)H, (14)N(n, (3)H)(12)C, and ternary fission (fission yield <0.01%)]. Typically, (3)H is present as tritiated water (HTO) and can become adsorbed into structural concrete from the surface inward where it will be held in a weakly bound form. However, a systematic analysis of a sequence of subsamples taken from a reactor bioshield using combustion and liquid scintillation analysis has identified two forms of (3)H, one weakly bound and one strongly bound. The strongly bound tritium, which originates from neutron capture on trace lithium ((6)Li) within mineral phases, requires temperatures in excess of 350 degrees C to achieve quantitative recovery. The weakly bound form of tritium can be liberated at significantly lower temperatures (100 degrees C) as HTO and is associated with dehydration of hydrous mineral components. Without an appreciation that two forms of tritium can exist in reactor bioshields, the (3)H content of samples may be severely underestimated using conventional analytical approaches. These findings exemplify the need to develop robust radioactive waste characterization procedures in support of nuclear decommissioning programs.

  19. A new scenario for the application of very intense lasers to nuclear fusion

    NASA Astrophysics Data System (ADS)

    Roso, Luis

    1996-11-01

    The ponderomotive motion of a charged particle inside a Terawatt-Petawatt laser pulse is studied. Based on a very simple classical model to account for the Coulomb repulsion, the possibility of nuclear collisions in the keV-MeV range is shown. Also, a simple analytical expression for the minimum internuclear distance is given. Since this range of energies is significant to trigger nuclear fusion reactions, this may result in an alternative approach to controlled fusion based on a non-thermalized plasma. The proposed system works for the deuterontriton fusion reaction, but is more appropriate for other reactions like the proton-7Li reaction, and also like the ecologically clean, boron-11B reaction.

  20. TENDL-2011: TALYS-based Evaluated Nuclear Data Library

    SciTech Connect

    Rochman, D.; Koning, A. J.

    2012-07-01

    The 4. release of the TENDL library, TENDL-2011 (TALYS-based Evaluated Nuclear Data Library) is described. This library consists of a complete set of nuclear reaction data for incident neutrons, photons, protons, deuterons, tritons, helions and alpha particles, from 10-5 eV up to 200 MeV, for all isotopes from {sup 6}Li to {sup 281}Ds that are either stable of have a half-life longer than 1 second. All data are completely and consistently evaluated using a software system consisting of the TALYS-1.2 nuclear reaction code, and other programs to handle resonance data, experimental data, data from existing evaluations, and to provide the final ENDF-6 formatting. The result is a nuclear data library with mutually consistent reaction information for all isotopes and a quality that increases with yearly updates. To produce this library, TALYS input parameters are adjusted for many nuclides so that calculated cross sections agree with experimental data, while for important nuclides experimental data are directly included. All information is available on www.talys.eu and www.talys.eu/TENDL-2011. (authors)

  1. Nuclear Halos

    SciTech Connect

    Vogt, Erich

    2010-07-27

    We show that extreme nuclear halos are caused only by pairs of s-wave neutrons (or single s-wave neutrons) and that such states occur much more frequently in the periodic table than previously believed. Besides lingering long near zero neutron separation energy such extreme halos have very remarkable properties: they can contribute significantly to the nuclear density at more than twice the normal nuclear radius and their spreading width can be very narrow. The properties of these states are primarily determined by the ''thickness'' of the nuclear surface in the mean-free nuclear potential and thus their importance increases greatly as we approach the neutron drip line. We discuss what such extreme halos are, where they occur, what their properties are and some of their impact on nuclear observations.

  2. Nuclear astrophysics

    SciTech Connect

    Haxton, W.C.

    1992-01-01

    The problem of core-collapse supernovae is used to illustrate the many connections between nuclear astrophysics and the problems nuclear physicists study in terrestrial laboratories. Efforts to better understand the collapse and mantle ejection are also motivated by a variety of interdisciplinary issues in nuclear, particle, and astrophysics, including galactic chemical evolution, neutrino masses and mixing, and stellar cooling by the emission of new particles. The current status of theory and observations is summarized.

  3. Nuclear astrophysics

    SciTech Connect

    Haxton, W.C.

    1992-12-31

    The problem of core-collapse supernovae is used to illustrate the many connections between nuclear astrophysics and the problems nuclear physicists study in terrestrial laboratories. Efforts to better understand the collapse and mantle ejection are also motivated by a variety of interdisciplinary issues in nuclear, particle, and astrophysics, including galactic chemical evolution, neutrino masses and mixing, and stellar cooling by the emission of new particles. The current status of theory and observations is summarized.

  4. Synthesis of 0.3Li2MnO3·0.7LiNi1/3Co1/3Mn1/3O2 cathode materials using 3-D urchin-like MnO2 as precursor for high performance lithium ion battery

    NASA Astrophysics Data System (ADS)

    Zhao, Chenhao; Hu, Zhibiao; Zhou, Yunlong; Fang, Shuzhen; Cai, Shaohan

    2015-02-01

    In the paper, we report synthesis of lithium rich layered oxide 0.3Li2MnO3·0.7LiNi1/3Co1/3Mn1/3O2 by using an urchin-like MnO2 as precursor. The influences of calcination temperatures on the structures and electrochemical performances of as-prepared materials are systematically studied. The results show that the obtained sample can partially retain the morphology of urchin-like precursor especially at low temperature, and a higher calcination temperature helps to improve the layered structure and particle size. As lithium ion battery cathodes, the 750 °C sample with the size of 100-200 nm reveals an optimal electrochemical performance. The initial discharge capacity of 234.6 mAh g-1 with high Coulombic efficiency of 84.6 % can be reached at 0.1C within 2.0-4.7 V. After 50 cycles, the capacity retention can reach 90.2 % at 0.5C. Even at high current density of 5C, the sample also shows a stable discharge capacity of 120.5 mAh g-1. Anyways, the urchin-like MnO2 directed route is suitable to prepare 0.3Li2MnO3·0.7LiNi1/3Co1/3Mn1/3O2 as lithium ion battery cathode.

  5. Nuclear Fission

    NASA Astrophysics Data System (ADS)

    Denschlag, J. O.

    This chapter first gives a survey on the history of the discovery of nuclear fission. It briefly presents the liquid-drop and shell models and their application to the fission process. The most important quantities accessible to experimental determination such as mass yields, nuclear charge distribution, prompt neutron emission, kinetic energy distribution, ternary fragment yields, angular distributions, and properties of fission isomers are presented as well as the instrumentation and techniques used for their measurement. The contribution concentrates on the fundamental aspects of nuclear fission. The practical aspects of nuclear fission are discussed in http://dx.doi.org/10.1007/978-1-4419-0720-2_57 of Vol. 6.

  6. Nuclear Safety

    SciTech Connect

    Silver, E G

    1989-01-01

    This document is a review journal that covers significant developments in the field of nuclear safety. Its scope includes the analysis and control of hazards associated with nuclear energy, operations involving fissionable materials, and the products of nuclear fission and their effects on the environment. Primary emphasis is on safety in reactor design, construction, and operation; however, the safety aspects of the entire fuel cycle, including fuel fabrication, spent-fuel processing, nuclear waste disposal, handling of radioisotopes, and environmental effects of these operations, are also treated.

  7. Measurement of hydrogen and lithium ion energy densities on PBFA II using direct nuclear activation diagnostics

    NASA Astrophysics Data System (ADS)

    Ruiz, C. L.; Cooper, G. W.; Chambers, G.; Schmidlapp, F. A.

    1997-01-01

    In the light-ion-beam fusion program at Sandia National Laboratories an intense lithium beam is being developed to drive inertial confinement fusion targets. An important issue is the purity of the beam. To assess this concern, direct nuclear activation diagnostics based on the reactions 7Li(p,n)7Be, 10B(p,α)7Be, and 19F(7Li,d)24Na were fielded to measure the energy densities of hydrogen and lithium in the beam. The hydrogen beam energy density was measured to be less than 2% of the lithium beam energy density on a majority (10) of the 19 LiF anode shots taken and was always less than 10%. The total hydrogen energy in the beam ranged from only 0.5-10 kJ. Over this shot series increasing efforts were made to clean the anode prior to each shot. In general, there was a modest reduction in the hydrogen energy fraction with improved cleaning, but no corresponding increase in the lithium energy density was seen. The lithium energy density as a function of location was also measured and found to typically vary by factors of 1.5-4 over the diode.

  8. Nuclear Threshold States: Yesterday, Today, Tomorrow

    SciTech Connect

    Ogloblin, A. A.; Danilov, A. N.; Demyanova, A. S.; Belyaeva, T. L.; Goncharov, S. A.

    2010-04-30

    50 years ago exotic nuclear states with abnormally large radii located close to the thresholds of emission of nucleons or clusters were predicted. Recently a hypothesis of possible existence of alpha-particle Bose condensation was proposed. The 0{sup +}{sub 2}(7.65 MeV) state of {sup 12}C(so-called Hoyle state) is considered to be the prototype of such condensed state and have a dilute structure. We propose two methods for searching the alpha-condensate signatures in the Hoyle state and some other ones near the alpha-thresholds by using inelastic diffractive and rainbow scattering. Inelastic scattering of {sup 2}H, {sup 3}He, {sup 4}He, {sup 6}Li, and {sup 12}C on {sup 12}C was studied and the enhancement of the {sup 12}C radius in the Hoyle state relatively the ground state radius by a factor of 1.2 was demonstrated. Another signature of the condensate structure, 70% probability of all three alpha-particles to be in the s-state, was observed for the Hoyle state by studying the {sup 8}Be transfer reaction. The analogs of the Hoyle state with enhanced radii were identified in {sup 11}B and {sup 13}C. The proposed methods of measuring the nuclear radii allowed observation of neutron halos in the excited states of {sup 9}Be and {sup 13}C. The conception of abnormal dimensions of the threshold states finds its confirmation in many nuclear phenomena both well-known and new ones. One of the perspective domains of its manifestation are the nuclei heavier than {sup 100}Sn with N = Z, which are able to emit several alpha particles.

  9. Nuclear safety

    NASA Technical Reports Server (NTRS)

    Buden, D.

    1991-01-01

    Topics dealing with nuclear safety are addressed which include the following: general safety requirements; safety design requirements; terrestrial safety; SP-100 Flight System key safety requirements; potential mission accidents and hazards; key safety features; ground operations; launch operations; flight operations; disposal; safety concerns; licensing; the nuclear engine for rocket vehicle application (NERVA) design philosophy; the NERVA flight safety program; and the NERVA safety plan.

  10. Nuclear privatization

    SciTech Connect

    Jeffs, E.

    1995-11-01

    The United Kingdom government announced in May 1995 plans to privatize the country`s two nuclear generating companies, Nuclear Electric and Scottish Nuclear. Under the plan, the two companies will become operating divisions of a unified holding company, to be called British Electric, with headquarters in Scotland. Britain`s nuclear plants were left out of the initial privatization in 1989 because the government believed the financial community would be unwilling to accept the open-ended liability of decommissioning the original nine stations based on the Magnox gas-cooled reactor. Six years later, the government has found a way around this by retaining these power stations in state ownership, leaving the new nuclear company with the eight Advanced Gas-cooled Reactor (AGR) stations and the recently completed Sizewell B PWR stations. The operating Magnox stations are to be transferred to BNFL, which operates two Magnox stations of their own at Calder Hall and Chapelcross.

  11. Nuclear materials

    SciTech Connect

    Not Available

    1992-08-01

    The Department of Energy (DOE) processes plutonium for use in nuclear weapons. This fact sheet responds to your September 6, 1991, request, that we describe the methods and facilities for DOE's plutonium processing. Plutonium, which is used to make nuclear weapons, does not exist in nature and has to be produced. However, DOE no longer produces plutonium for use in nuclear weapons. Instead, DOE processes and recycles the plutonium from retired nuclear weapons and the plutonium that remains as scrap or residue from plutonium processing. This paper reports that DOE recovers plutonium through two basic processes-aqueous and pyrochemical-at four processing sites-Rocky Flats, Savannah River, Hanford, and Los Alamos. However, because of environmental and safety concerns and reductions in nuclear weapons, DOE has closed or may close most of the processing facilities. Only Los Alamos' processing facilities are currently operating.

  12. Manufacturing of calcium, lithium and molybdenum targets for use in nuclear physics experiments

    NASA Astrophysics Data System (ADS)

    Kheswa, N. Y.; Papka, P.; Buthelezi, E. Z.; Lieder, R. M.; Neveling, R.; Newman, R. T.

    2010-02-01

    This paper describes methods used in the manufacturing of chemically reactive targets such as calcium ( natCa), lithium-6 ( 6Li) and molybdenum-97 ( 97Mo) for nuclear physics experiments at the iThemba LABS cyclotron facility (Faure, South Africa). Due to the chemical properties of these materials a suitable and controlled environment was established in order to minimize oxygen contamination of targets. Calcium was prepared by means of vacuum evaporation while lithium was cold rolled to a desired thickness. In the case of molybdenum, the metallic powder was melted under vacuum using an e-gun followed by cold rolling of the metal bead to a desired thickness. In addition, latest developments toward the establishment of a dedicated nuclear physics target laboratory are discussed.

  13. Li isotope fractionation in aragonite precipitated from seawater at different rates

    NASA Astrophysics Data System (ADS)

    Gabitov, R. I.; Schmitt, A. K.; Gaetani, G. A.; Cohen, A. L.; Watson, E. B.; Rosner, M.

    2009-12-01

    The marine carbonates retain 7Li/6Li signatures of seawater and may record fluctuations in global hydrothermal fluid circulation or weathering rate of continental rocks. The development of a 7Li/6Li paleoproxy requires evaluating the influence of environmental parameters such as seawater composition and growth kinetics on 7Li/6Li fractionation in carbonates. A number of studies suggest that 7Li/6Li of biogenic and abiogenic aragonite is not affected by temperature, salinity, pH, or pCO2 (Marriott et al. 2004 a,b; Rollion-Bar et al. 2009). However, the influence of aragonite precipitation rate on 7Li/6Li fractionation has not been evaluated. We have carried out aragonite precipitation experiments to investigate this, and found that 7Li/6Li increases by up to ~4‰ as precipitation rate increases from 0.3 to 20 µmol/min. Bulk Li isotope analyses of two aragonite samples and corresponding fluids were performed using a Thermo Scientific NEPTUNE MC-ICP-MS at WHOI. In situ measurements of the same samples were conducted with the CAMECA ims 1270 ion microprobe at UCLA; two glass standards NIST-612 and 614 were analyzed for assessing instrumental reproducibility. Ion probe analyses were performed a 2-5 nA 16O- primary beam with 25-30 µm lateral dimensions. 7Li/6Li ratios were measured by peak switching. Single spot analyses consisted of 60-72 cycles with counting times for 6Li and 7Li of 10 and 4 seconds, respectively. Each spot was pre-sputtered until 7Li/6Li reached a steady-state value. Average ion microprobe instrumental mass fractionations for 7Li/6Li are approximately -3 and +12 ‰ for aragonite and silicate glass respectively. Our results suggest a positive relationship between aragonite precipitation rate and 7Li/6Li fractionation. Bulk (ICP-MS) measurements indicate that 7Li/6Li increased by ~2 ‰ with increasing precipitation rate of aragonite from 0.3 to 20 µmol/min. The intra-sample standard deviation (SD) was <0.8‰. The mass of aragonite precipitated in

  14. Fabrication and electrochemical performance of 0.6Li2MnO3-0.4Li(Ni1/3Co1/3Mn1/3)O2 microspheres by two-step spray-drying process

    PubMed Central

    Son, Mun Yeong; Lee, Jung-Kul; Kang, Yun Chan

    2014-01-01

    0.6Li2MnO3–0.4Li(Ni1/3Co1/3Mn1/3)O2 composite microspheres with dense structures are prepared by a two-step spray-drying process. Precursor powders with hollow and porous structures prepared by the spray-drying process are post-treated at a low temperature of 400°C and then wet-milled to obtain a slurry with high stability. The slurry of the mixture of metal oxides is spray-dried to prepare precursor aggregate powders several microns in size. Post-treatment of these powders at high temperatures (>700°C) produces 0.6Li2MnO3–0.4Li(Ni1/3Co1/3Mn1/3)O2 composite microspheres with dense structures and high crystallinity. The mean size and geometric standard deviation of the composite microspheres post-treated at 900°C are 4 μm and 1.38, respectively. Further, the initial charge capacities of the aggregated microspheres post-treated at 700, 800, 900, and 1000°C are 336, 349, 383, and 128 mA h g−1, respectively, and the corresponding discharge capacities are 286, 280, 302, and 77 mA h g−1, respectively. The discharge capacity of the composite microspheres post-treated at an optimum temperature of 900°C after 100 cycles is 242 mA h g−1, and the corresponding capacity retention is 80%. PMID:25168912

  15. Li2ZrO3-coated 0.4Li2MnO3·0.6LiNi1/3Co1/3Mn1/3O2 for high performance cathode material in lithium-ion battery

    NASA Astrophysics Data System (ADS)

    Miao, Xiaowei; Ni, Huan; Zhang, Han; Wang, Chunguang; Fang, Jianhui; Yang, Gang

    2014-10-01

    To improve the high-rate capacity and cycle ability, minor Li2ZrO3 successfully coat the nanoparticles of 0.4Li2MnO3·0.6LiNi1/3Co1/3Mn1/3O2 (LMO) via sol-gel method. The crystal structure and electrochemical properties of the bare and coated material are studied by X-ray diffractometry (XRD), transmission electron microscopy (TEM), cyclic voltammetry (CV), galvanostatic intermittent titration technique (GITT), and charge-discharge tests. The lithium diffusion coefficient of LMO increases one to two orders of magnitude after Li2ZrO3 coating. Li2ZrO3 coating improves the rate capability and cycling stability of LMO. Within the cut-off voltage of 2.5-4.8 V, the initial discharge capacity of Li2ZrO3-coated 0.4Li2MnO3·0.6LiNi1/3Co1/3Mn1/3O2 (LZO-LMO) reaches to 264 mAh g-1 at 0.1 C rate, and the capacity remains 235 mAh g-1 after 100 cycles. At the current rates of 1, 2, 5 and 10 C, the maximum discharge capacities of LZO-LMO are 205.6, 161, 153.8 and 106 mAh g-1, respectively. Minor Li2ZrO3 modification plays an important role to enhance the high-rate capability and cycle ability of LMO.

  16. Light elements synthesized in the He-layer and the H-rich envelope of a type II supernova -- Influence of the adopted neutrino emission model

    NASA Astrophysics Data System (ADS)

    Yoshida, T.; Emori, H.; Nakazawa, K.

    2000-03-01

    In order to establish a suitable manner for finding presolar grains of supernova origin, we simulated the explosive nucleosynthesis of light elements, i.e., CNO-elements and X-elements (Li, Be, and B), in the He-layer and the H-rich envelope of a 16.2 M⊙ supernova and calculated their final abundances and abundance ratios using the nuclear reaction network. We also investigated the response of the synthesized abundances of light elements to the change of strength and duration of the neutrino emission, about which we have not a precise knowledge. The obtained results are as follows. The amounts of 6Li and 9Be produced during the supernova explosion are quite small. The ratios of 6Li/7Li and 9Be/7Li are less than 2 × 10-4, which are much smaller than the corresponding solar-system values. The other X-elements and CNO-elements (except 12C and 16O) are synthesized, more or less, and their abundances depend strongly on the internal mass coordinate as well as the adopted neutrino emission model. However, 11B/7Li ratio and isotopic ratios of CNO-elements are confined within one order of magnitude or so. On the basis of the above results, we finally proposed useful diagrams between two isotopic (elemental) ratios, which would help us to find presolar grains of supernova origin.

  17. Magnetic-field effects in transitions of X Li molecules (X: even isotopes of group II atoms)

    SciTech Connect

    Gopakumar, Geetha; Abe, Minori; Hada, Masahiko; Kajita, Masatoshi

    2011-10-15

    We analyze the Zeeman shift in the (v,N)=(0,0){yields}(1,0) transition frequency of X Li molecules (X: even isotopes of group II atoms), which is of interest in metrology. The Zeeman shift in the transition frequency between stretching states is found to be less than 1 mHz with a magnetic field of 1 G. X {sup 6}Li molecules are more advantageous than X {sup 7}Li molecules for measuring the transition frequency without the Zeeman shift because of the smaller g factor of the Li nuclear spin.

  18. Nuclear Speckles

    PubMed Central

    Spector, David L.; Lamond, Angus I.

    2011-01-01

    Nuclear speckles, also known as interchromatin granule clusters, are nuclear domains enriched in pre-mRNA splicing factors, located in the interchromatin regions of the nucleoplasm of mammalian cells. When observed by immunofluorescence microscopy, they usually appear as 20–50 irregularly shaped structures that vary in size. Speckles are dynamic structures, and their constituents can exchange continuously with the nucleoplasm and other nuclear locations, including active transcription sites. Studies on the composition, structure, and dynamics of speckles have provided an important paradigm for understanding the functional organization of the nucleus and the dynamics of the gene expression machinery. PMID:20926517

  19. Nuclear reprogramming.

    PubMed

    Halley-Stott, Richard P; Pasque, Vincent; Gurdon, J B

    2013-06-01

    There is currently particular interest in the field of nuclear reprogramming, a process by which the identity of specialised cells may be changed, typically to an embryonic-like state. Reprogramming procedures provide insight into many mechanisms of fundamental cell biology and have several promising applications, most notably in healthcare through the development of human disease models and patient-specific tissue-replacement therapies. Here, we introduce the field of nuclear reprogramming and briefly discuss six of the procedures by which reprogramming may be experimentally performed: nuclear transfer to eggs or oocytes, cell fusion, extract treatment, direct reprogramming to pluripotency and transdifferentiation.

  20. ENDF/B-VII.0: Next Generation Evaluated Nuclear Data Library for Nuclear Science and Technology

    SciTech Connect

    Chadwick, M B; Oblozinsky, P; Herman, M; Greene, N M; McKnight, R D; Smith, D L; Young, P G; MacFarlane, R E; Hale, G M; Haight, R C; Frankle, S; Kahler, A C; Kawano, T; Little, R C; Madland, D G; Moller, P; Mosteller, R; Page, P; Talou, P; Trellue, H; White, M; Wilson, W B; Arcilla, R; Dunford, C L; Mughabghab, S F; Pritychenko, B; Rochman, D; Sonzogni, A A; Lubitz, C; Trumbull, T H; Weinman, J; Brown, D; Cullen, D E; Heinrichs, D; McNabb, D; Derrien, H; Dunn, M; Larson, N M; Leal, L C; Carlson, A D; Block, R C; Briggs, B; Cheng, E; Huria, H; Kozier, K; Courcelle, A; Pronyaev, V; der Marck, S

    2006-10-02

    We describe the next generation general purpose Evaluated Nuclear Data File, ENDF/B-VII.0, of recommended nuclear data for advanced nuclear science and technology applications. The library, released by the U.S. Cross Section Evaluation Working Group (CSEWG) in December 2006, contains data primarily for reactions with incident neutrons, protons, and photons on almost 400 isotopes. The new evaluations are based on both experimental data and nuclear reaction theory predictions. The principal advances over the previous ENDF/B-VI library are the following: (1) New cross sections for U, Pu, Th, Np and Am actinide isotopes, with improved performance in integral validation criticality and neutron transmission benchmark tests; (2) More precise standard cross sections for neutron reactions on H, {sup 6}Li, {sup 10}B, Au and for {sup 235,238}U fission, developed by a collaboration with the IAEA and the OECD/NEA Working Party on Evaluation Cooperation (WPEC); (3) Improved thermal neutron scattering; (4) An extensive set of neutron cross sections on fission products developed through a WPEC collaboration; (5) A large suite of photonuclear reactions; (6) Extension of many neutron- and proton-induced reactions up to an energy of 150 MeV; (7) Many new light nucleus neutron and proton reactions; (8) Post-fission beta-delayed photon decay spectra; (9) New radioactive decay data; and (10) New methods developed to provide uncertainties and covariances, together with covariance evaluations for some sample cases. The paper provides an overview of this library, consisting of 14 sublibraries in the same, ENDF-6 format, as the earlier ENDF/B-VI library. We describe each of the 14 sublibraries, focusing on neutron reactions. Extensive validation, using radiation transport codes to simulate measured critical assemblies, show major improvements: (a) The long-standing underprediction of low enriched U thermal assemblies is removed; (b) The {sup 238}U, {sup 208}Pb, and {sup 9}Be reflector

  1. (Nuclear theory). [Research in nuclear physics

    SciTech Connect

    Haxton, W.

    1990-01-01

    This report discusses research in nuclear physics. Topics covered in this paper are: symmetry principles; nuclear astrophysics; nuclear structure; quark-gluon plasma; quantum chromodynamics; symmetry breaking; nuclear deformation; and cold fusion. (LSP)

  2. Current Status of Nuclear Physics Research

    NASA Astrophysics Data System (ADS)

    Bertulani, Carlos A.; Hussein, Mahir S.

    2015-12-01

    In this review, we discuss the current status of research in nuclear physics which is being carried out in different centers in the world. For this purpose, we supply a short account of the development in the area which evolved over the last nine decades, since the discovery of the neutron. The evolution of the physics of the atomic nucleus went through many stages as more data became available. We briefly discuss models introduced to discern the physics behind the experimental discoveries, such as the shell model, the collective model, the statistical model, the interacting boson model, etc., some of these models may be seemingly in conflict with each other, but this was shown to be only apparent. The richness of the ideas and abundance of theoretical models attests to the important fact that the nucleus is a really singular system in the sense that it evolves from two-body bound states such as the deuteron, to few-body bound states, such as 4He, 7Li, 9Be, etc. and up the ladder to heavier bound nuclei containing up to more than 200 nucleons. Clearly, statistical mechanics, usually employed in systems with very large number of particles, would seemingly not work for such finite systems as the nuclei, neither do other theories which are applicable to condensed matter. The richness of nuclear physics stems from these restrictions. New theories and models are presently being developed. Theories of the structure and reactions of neutron-rich and proton-rich nuclei, called exotic nuclei, halo nuclei, or Borromean nuclei, deal with the wealth of experimental data that became available in the last 35 years. Furthermore, nuclear astrophysics and stellar and Big Bang nucleosynthesis have become a more mature subject. Due to limited space, this review only covers a few selected topics, mainly those with which the authors have worked on. Our aimed potential readers of this review are nuclear physicists and physicists in other areas, as well as graduate students interested in

  3. Nuclear battlefields

    SciTech Connect

    Arkin, W.M.; Fieldhouse, R.W.

    1985-01-01

    This book provides complete data on the nuclear operations and research facilities in the U.S.A., the U.S.S.R., France, China and the U.K. It describes detailed estimates on the U.S.S.R.'s nuclear stockpile for over 500 locations. It shows how non-nuclear countries cooperate with the world-wide war machine. And it maps the U.S. nuclear facilities from Little America, WY, and Charleston, SC, to the battleships patroling the world's oceans and subs stalking under the sea. The data were gathered from unclassified sources through the Freedom of Information Act, from data supplied to military installations, and from weapons source books. It provides guidance for policymakers, government and corporate officials.

  4. NUCLEAR REACTOR

    DOEpatents

    Sherman, J.; Sharbaugh, J.E.; Fauth, W.L. Jr.; Palladino, N.J.; DeHuff, P.G.

    1962-10-23

    A nuclear reactor incorporating seed and blanket assemblies is designed. Means are provided for obtaining samples of the coolant from the blanket assemblies and for varying the flow of coolant through the blanket assemblies. (AEC)

  5. Nuclear Disarmament.

    ERIC Educational Resources Information Center

    Johnson, Christopher

    1982-01-01

    Material about nuclear disarmament and the arms race should be included in secondary school curricula. Teachers can present this technical, controversial, and frightening material in a balanced and comprehensible way. Resources for instructional materials are listed. (PP)

  6. Nuclear Nonproliferation

    SciTech Connect

    Atkins-Duffin, C E

    2008-12-10

    With an explosion equivalent of about 20kT of TNT, the Trinity test was the first demonstration of a nuclear weapon. Conducted on July 16, 1945 in Alamogordo, NM this site is now a Registered National Historic Landmark. The concept and applicability of nuclear power was demonstrated on December 20, 1951 with the Experimental Breeder Reactor Number One (EBR-1) lit four light bulbs. This reactor is now a Registered National Historic Landmark, located near Arco, ID. From that moment forward it had been clearly demonstrated that nuclear energy has both peaceful and military applications and that the civilian and military fuel cycles can overlap. For the more than fifty years since the Atoms for Peace program, a key objective of nuclear policy has been to enable the wider peaceful use of nuclear energy while preventing the spread of nuclear weapons. Volumes have been written on the impact of these two actions on the world by advocates and critics; pundits and practioners; politicians and technologists. The nations of the world have woven together a delicate balance of treaties, agreements, frameworks and handshakes that are representative of the timeframe in which they were constructed and how they have evolved in time. Collectively these vehicles attempt to keep political will, nuclear materials and technology in check. This paper captures only the briefest abstract of the more significant aspects on the Nonproliferation Regime. Of particular relevance to this discussion is the special nonproliferation sensitivity associated with the uranium isotope separation and spent fuel reprocessing aspects of the nuclear fuel cycle.

  7. Nuclear Data

    SciTech Connect

    White, Morgan C.

    2014-01-23

    PowerPoint presentation targeted for educational use. Nuclear data comes from a variety of sources and in many flavors. Understanding where the data you use comes from and what flavor it is can be essential to understand and interpret your results. This talk will discuss the nuclear data pipeline with particular emphasis on providing links to additional resources that can be used to explore the issues you will encounter.

  8. Nuclear cardiac

    SciTech Connect

    Slutsky, R.; Ashburn, W.L.

    1982-01-01

    The relationship between nuclear medicine and cardiology has continued to produce a surfeit of interesting, illuminating, and important reports involving the analysis of cardiac function, perfusion, and metabolism. To simplify the presentation, this review is broken down into three major subheadings: analysis of myocardial perfusion; imaging of the recent myocardial infarction; and the evaluation of myocardial function. There appears to be an increasingly important relationship between cardiology, particularly cardiac physiology, and nuclear imaging techniques. (KRM)

  9. Nuclear accidents

    SciTech Connect

    Mobley, J.A.

    1982-05-01

    A nuclear accident with radioactive contamination can happen anywhere in the world. Because expert nuclear emergency teams may take several hours to arrive at the scene, local authorities must have a plan of action for the hours immediately following an accident. The site should be left untouched except to remove casualties. Treatment of victims includes decontamination and meticulous wound debridement. Acute radiation syndrome may be an overwhelming sequela.

  10. Transverse Isotropy: Disappearance of Mott oscillations in sub-barrier elastic scattering of identical heavy ions and the nuclear ineraction

    NASA Astrophysics Data System (ADS)

    Hussein, Mahir; Canto, L. Felipe; Donangelo, Raul

    2015-04-01

    It is found that at a certain critical value of the Sommerfeld parameter the Mott oscillations usually present in the scattering of identical heavy ions, disappear and the cross section becomes quite flat. We call this effect Transverse Isotropy (TI) (L. F. Canto, R. Donangelo and M. S. Hussein, Mod. Phys. Lett. A, 16), 1027 (2001). The critical value of the Sommerfeld parameter at which TI sets in is found to be ηc =√{ 3 s + 2 } , where s is the spin of the nuclei participating in the scattering. No TI is found in the Mott scattering of identical Fermionic nuclei. The critical center of mass energy corresponding to ηc is found to be Ec = 0.40 MeV for α + α (s = 0), and 1.2 MeV for 6 Li + 6 LI (s = 1). We further found that the inclusion of the nuclear interaction induces a significant modification in the TI. This can be verified by calculating the second derivative of the cross section at θ =90° . We suggest measurements at these sub-barrier energies for the purpose of extracting useful information about the nuclear interaction between light heavy ions. Supported by CNPq, FAPESP, FAPERJ, CAPES/ITA.

  11. Nuclear telemedicine

    NASA Astrophysics Data System (ADS)

    Morrison, R. T.; Szasz, I. J.

    1990-06-01

    Diagnostic nuclear medicine patient images have been transniitted for 8 years from a regional conununity hospital to a university teaching hospital 700 kiloinetres away employing slow scan TV and telephone. Transruission and interpretation were done at the end of each working day or as circumstances required in cases of emergencies. Referring physicians received the nuclear medicine procedure report at the end of the completion day or within few minutes of completion in case of emergency procedures. To date more than 25 patient studies have been transmitted for interpretation. Blinded reinterpretation of the original hard copy data of 350 patient studies resulted in 100 agreement with the interpretation of transmitted data. This technique provides high quality diagnostic and therapeutic nuclear medicine services in remote hospitals where the services of an on-site nuclear physician is not available. 2. HISTORY Eight years ago when the nuclear medicine physician at Trail Regional Hospital left the Trail area and an other could not be recruited we examined the feasibility of image transmission by phone for interpretation since closing the department would have imposed unacceptable physical and financial hardship and medical constraints on the patient population the nearest nuclear medicine facility was at some 8 hours drive away. In hospital patients would have to be treated either based purely on physical findings or flown to Vancouver at considerable cost to the health care system (estimated cost $1500.

  12. Polarization effects in the quasielastic ( p, 2 p) reaction with the nuclear S-Shell Protons at 1 GeV

    NASA Astrophysics Data System (ADS)

    Miklukho, O. V.; Kisselev, A. Yu.; Aksenov, D. A.; Amalsky, G. M.; Andreev, V. A.; Evstiukhin, S. V.; Fedorov, O. Ya.; Gavrilov, G. E.; Izotov, A. A.; Kochenda, L. M.; Levchenko, M. P.; Maysuzenko, D. A.; Murzin, V. A.; Novinsky, D. V.; Prokofiev, A. N.; Shvedchikov, A. V.; Trautman, V. Yu.; Trush, S. I.; Zhdanov, A. A.

    2013-07-01

    The polarization of the secondary protons in the ( p, 2 p) reaction with the S-shell protons of nuclei 4He, 6Li, 12C, 28Si, 40Ca was measured at 1 GeV unpolarized proton beam. The spin correlation parameters C ij for the 4He and 12C targets also were for the first time obtained as well. The polarization measurements were performed by means of a two-arm magnetic spectrometer, each arm of which was equipped with the multiwire-proportional chamber polarimeter. This experiment was aimed to study a modification of the proton-proton scattering matrix in the nuclear medium.

  13. Single-Crystal Time-of-Flight Neutron Diffraction and Magic-Angle-Spinning NMR Spectroscopy Resolve the Structure and (1)H and (7)Li Dynamics of the Uranyl Peroxide Nanocluster U60.

    PubMed

    Olds, Travis A; Dembowski, Mateusz; Wang, Xiaoping; Hoffman, Christina; Alam, Todd M; Hickam, Sarah; Pellegrini, Kristi L; He, Junhong; Burns, Peter C

    2017-08-21

    Single-crystal time-of-flight neutron diffraction has provided atomic resolution of H atoms of H2O molecules and hydroxyl groups, as well as Li cations in the uranyl peroxide nanocluster U60. Solid-state magic-angle-spinning nuclear magnetic resonance (MAS NMR) spectroscopy was used to confirm the dynamics of these constituents, revealing the transportation of Li atoms and H2O through cluster walls. H atoms of hydroxyl units that are located on the cluster surface are involved in the transfer of H2O and Li cations from inside to outside and vice versa. This exchange occurs as a concerted motion and happens rapidly even in the solid state. As a consequence of its large size and open hexagonal pores, U60 exchanges Li cations more rapidly compared to other uranyl nanoclusters.

  14. ENDF/B-VII.0: Next Generation Evaluated Nuclear Data Library for Nuclear Science and Technology

    NASA Astrophysics Data System (ADS)

    Chadwick, M. B.; Obložinský, P.; Herman, M.; Greene, N. M.; McKnight, R. D.; Smith, D. L.; Young, P. G.; MacFarlane, R. E.; Hale, G. M.; Frankle, S. C.; Kahler, A. C.; Kawano, T.; Little, R. C.; Madland, D. G.; Moller, P.; Mosteller, R. D.; Page, P. R.; Talou, P.; Trellue, H.; White, M. C.; Wilson, W. B.; Arcilla, R.; Dunford, C. L.; Mughabghab, S. F.; Pritychenko, B.; Rochman, D.; Sonzogni, A. A.; Lubitz, C. R.; Trumbull, T. H.; Weinman, J. P.; Brown, D. A.; Cullen, D. E.; Heinrichs, D. P.; McNabb, D. P.; Derrien, H.; Dunn, M. E.; Larson, N. M.; Leal, L. C.; Carlson, A. D.; Block, R. C.; Briggs, J. B.; Cheng, E. T.; Huria, H. C.; Zerkle, M. L.; Kozier, K. S.; Courcelle, A.; Pronyaev, V.; van der Marck, S. C.

    2006-12-01

    We describe the next generation general purpose Evaluated Nuclear Data File, ENDF/B-VII.0, of recommended nuclear data for advanced nuclear science and technology applications. The library, released by the U.S. Cross Section Evaluation Working Group (CSEWG) in December 2006, contains data primarily for reactions with incident neutrons, protons, and photons on almost 400 isotopes, based on experimental data and theory predictions. The principal advances over the previous ENDF/B-VI library are the following: (1) New cross sections for U, Pu, Th, Np and Am actinide isotopes, with improved performance in integral validation criticality and neutron transmission benchmark tests; (2) More precise standard cross sections for neutron reactions on H, 6Li, 10B, Au and for 235,238U fission, developed by a collaboration with the IAEA and the OECD/NEA Working Party on Evaluation Cooperation (WPEC); (3) Improved thermal neutron scattering; (4) An extensive set of neutron cross sections on fission products developed through a WPEC collaboration; (5) A large suite of photonuclear reactions; (6) Extension of many neutron- and proton-induced evaluations up to 150 MeV; (7) Many new light nucleus neutron and proton reactions; (8) Post-fission beta-delayed photon decay spectra; (9) New radioactive decay data; (10) New methods for uncertainties and covariances, together with covariance evaluations for some sample cases; and (11) New actinide fission energy deposition. The paper provides an overview of this library, consisting of 14 sublibraries in the same ENDF-6 format as the earlier ENDF/B-VI library. We describe each of the 14 sublibraries, focusing on neutron reactions. Extensive validation, using radiation transport codes to simulate measured critical assemblies, show major improvements: (a) The long-standing underprediction of low enriched uranium thermal assemblies is removed; (b) The 238U and 208Pb reflector biases in fast systems are largely removed; (c) ENDF/B-VI.8 good

  15. Nuclear risk

    SciTech Connect

    Levenson, M.

    1989-01-01

    The title of our session, Nuclear Risk Versus Other Power Options, is provocative. It is also a title with different meanings to different people. To the utility chief executive officer, nuclear power is a high-risk financial undertaking because of political and economic barriers to cost recovery. To the utility dispatcher, it is a high-risk future power source since plant completion and start-up dates can be delayed for very long times due to uncertain legal and political issues. To the environmentalist, concerned about global effects such as greenhouse and acid rain, nuclear power is a relatively low risk energy source. To the financial people, nuclear power is a cash cow turned sour because of uncertainties as to what new plants will cost and whether they will even be allowed to operate. The statistics on risk are known and the results of probability risk assessment calculations of risks are known. The challenge is not to make nuclear power safer, it is already one of the safest, if not the safest, source of power currently available. The challenge is to find a way to communicate this to the public.

  16. Nuclear Reaction Recoil Fragments as Probes of Electronic Structure in Condensed Matter.

    NASA Astrophysics Data System (ADS)

    Bishop, Judith Lance

    Ambiguities in the stopping powers of many solids are frequently observed. When the cross-sections for constituent atoms are reliable, the deviations can be discussed meaningfully. This work measures cross-sections for boron, hexagonal boron -nitride, cubic boron-nitride (borazon) and cubic boron -phosphide and suggests that these samples may provide reasonable atomic cross-sections. Intermolecular deviations may exist, but molecular deviations appear to be absent. The method used for measuring cross-sections is based on information obtained from radiating Li('7) projectiles, whose motion and internal excitation are initiated by the thermal nuclear reaction ('10)B(n,(alpha))('7)Li* These projectiles have well defined initial momentum and spend their entire lives confined to the stopping medium.

  17. Nuclear-reaction recoil fragments as probes of electronic structure in condensed matter

    SciTech Connect

    Bishop, J.L.

    1986-01-01

    Ambiguities in the stopping powers of many solids are frequently observed. When the cross-sections for constituent atoms are reliable, the deviations can be discussed meaningfully. This work measures cross-sections for boron, hexagonal boron-nitride, cubic boron-nitride (borazon) and cubic boron-phosphide and suggests that these samples may provide reasonable atomic cross-sections. Intermolecular deviations may exist, but molecular deviations appear to be absent. The method used for measuring cross-sections is based on information obtained from radiating Li{sup 7} projectiles, whose motion and internal excitation are initiated by the thermal nuclear reaction {sup 10}B(n,{alpha}){sup 7}Li{sup *}. These projectiles have well defined initial momentum and spend their entire lives confined to the stopping medium.

  18. Nuclear scales

    SciTech Connect

    Friar, J.L.

    1998-12-01

    Nuclear scales are discussed from the nuclear physics viewpoint. The conventional nuclear potential is characterized as a black box that interpolates nucleon-nucleon (NN) data, while being constrained by the best possible theoretical input. The latter consists of the longer-range parts of the NN force (e.g., OPEP, TPEP, the {pi}-{gamma} force), which can be calculated using chiral perturbation theory and gauged using modern phase-shift analyses. The shorter-range parts of the force are effectively parameterized by moments of the interaction that are independent of the details of the force model, in analogy to chiral perturbation theory. Results of GFMC calculations in light nuclei are interpreted in terms of fundamental scales, which are in good agreement with expectations from chiral effective field theories. Problems with spin-orbit-type observables are noted.

  19. Nuclear astrophysics

    SciTech Connect

    Penionzhkevich, Yu. E.

    2010-08-15

    The International Year of Astronomy 2009 (IYA2009) was declared by the 62nd General Assembly of the United Nations and was also endorsed by UNESCO. Investigations in the realms of particle and nuclear physicsmake a large contribution in the development of our ideas of the properties of the Universe. The present article discusses some problems of the evolution of the Universe, nucleosyntheses, and cosmochronology from the point of view of nuclear and particle physics. Processes occurring in the Universe are compared with the mechanisms of the production and decay of nuclei, as well as with the mechanisms of their interaction at high energies. Examples that demonstrate the potential of nuclearphysics methods for studying cosmic objects and the properties of the Universe are given. The results that come from investigations into nuclear reactions induced by beams of radioactive nuclei and which make it possible to take a fresh look at the nucleosynthesis scenario in the range at light nuclei are presented.

  20. Nuclear waste

    SciTech Connect

    Not Available

    1988-05-01

    This paper discusses how, as part of the Department of Energy's implementation of the Nuclear Waste Policy Act of 1982, DOE is required to investigate a site at Yucca Mountain, Nevada and, if it determines that the site is suitable, recommend to the President its selection for a nuclear waste repository. The Nuclear Regulatory Commission, in considering development of the plan, issued five objections, one of which is DOE's failure to recognize the range of alternative conceptual models of the Yucca Mountain site that can be supported by the limited existing technical data. At the end of the quarter DOE directed its project offices in Washington and Texas to begin orderly phase-out of all site-specific repository activities. Costs for this phase-out are $53 million for the Deaf Smith site and $85 million for the Hanford site.

  1. Nuclear Models

    NASA Astrophysics Data System (ADS)

    Fossión, Rubén

    2010-09-01

    The atomic nucleus is a typical example of a many-body problem. On the one hand, the number of nucleons (protons and neutrons) that constitute the nucleus is too large to allow for exact calculations. On the other hand, the number of constituent particles is too small for the individual nuclear excitation states to be explained by statistical methods. Another problem, particular for the atomic nucleus, is that the nucleon-nucleon (n-n) interaction is not one of the fundamental forces of Nature, and is hard to put in a single closed equation. The nucleon-nucleon interaction also behaves differently between two free nucleons (bare interaction) and between two nucleons in the nuclear medium (dressed interaction). Because of the above reasons, specific nuclear many-body models have been devised of which each one sheds light on some selected aspects of nuclear structure. Only combining the viewpoints of different models, a global insight of the atomic nucleus can be gained. In this chapter, we revise the the Nuclear Shell Model as an example of the microscopic approach, and the Collective Model as an example of the geometric approach. Finally, we study the statistical properties of nuclear spectra, basing on symmetry principles, to find out whether there is quantum chaos in the atomic nucleus. All three major approaches have been rewarded with the Nobel Prize of Physics. In the text, we will stress how each approach introduces its own series of approximations to reduce the prohibitingly large number of degrees of freedom of the full many-body problem to a smaller manageable number of effective degrees of freedom.

  2. Nuclear Models

    SciTech Connect

    Fossion, Ruben

    2010-09-10

    The atomic nucleus is a typical example of a many-body problem. On the one hand, the number of nucleons (protons and neutrons) that constitute the nucleus is too large to allow for exact calculations. On the other hand, the number of constituent particles is too small for the individual nuclear excitation states to be explained by statistical methods. Another problem, particular for the atomic nucleus, is that the nucleon-nucleon (n-n) interaction is not one of the fundamental forces of Nature, and is hard to put in a single closed equation. The nucleon-nucleon interaction also behaves differently between two free nucleons (bare interaction) and between two nucleons in the nuclear medium (dressed interaction).Because of the above reasons, specific nuclear many-body models have been devised of which each one sheds light on some selected aspects of nuclear structure. Only combining the viewpoints of different models, a global insight of the atomic nucleus can be gained. In this chapter, we revise the the Nuclear Shell Model as an example of the microscopic approach, and the Collective Model as an example of the geometric approach. Finally, we study the statistical properties of nuclear spectra, basing on symmetry principles, to find out whether there is quantum chaos in the atomic nucleus. All three major approaches have been rewarded with the Nobel Prize of Physics. In the text, we will stress how each approach introduces its own series of approximations to reduce the prohibitingly large number of degrees of freedom of the full many-body problem to a smaller manageable number of effective degrees of freedom.

  3. Nuclear pursuits

    SciTech Connect

    Not Available

    1993-05-01

    This table lists quantities of warheads (in stockpile, peak number per year, total number built, number of known test explosions), weapon development milestones (developers of the atomic bomb and hydrogen bomb, date of first operational ICBM, first nuclear-powered naval SSN in service, first MIRVed missile deployed), and testing milestones (first fission test, type of boosted fission weapon, multistage thermonuclear test, number of months from fission bomb to multistage thermonuclear bomb, etc.), and nuclear infrastructure (assembly plants, plutonium production reactors, uranium enrichment plants, etc.). Countries included in the tally are the United States, Soviet Union, Britain, France, and China.

  4. Nuclear winter or nuclear fall?

    NASA Astrophysics Data System (ADS)

    Berger, André

    Climate is universal. If a major modern nuclear war (i.e., with a large number of small-yield weapons) were to happen, it is not even necessary to have a specific part of the world directly involved for there to be cause to worry about the consequences for its inhabitants and their future. Indeed, smoke from fires ignited by the nuclear explosions would be transported by winds all over the world, causing dark and cold. According to the first study, by Turco et al. [1983], air surface temperature over continental areas of the northern mid-latitudes (assumed to be the nuclear war theatre) would fall to winter levels even in summer (hence the term “nuclear winter”) and induce drastic climatic conditions for several months at least. The devastating effects of a nuclear war would thus last much longer than was assumed initially. Discussing to what extent these estimations of long-term impacts on climate are reliable is the purpose of this article.

  5. Determination of lithium isotopes at natural abundance levels by atomic absorption spectrometry

    USGS Publications Warehouse

    Meier, A.L.

    1982-01-01

    The relationships of the absorption of 6Li and 7Li hollow cathode lamp emissions are used to determine lithium isotopic composition in the natural abundance range of geologic materials. Absorption was found to have a nonlinear dependence upon total lithium concentration and isotopic composition. A method using nonlinear equations to describe the relationship of the absorption of 6Li and 7Li lamp radiation is proposed as a means of calculating isotopic composition that is independent of total lithium concentration.

  6. Lithium isotopes: differential effects on renal function and histology.

    PubMed

    Stoll, P M; Stokes, P E; Okamoto, M

    2001-08-01

    Reduction in renal concentrating ability has been reported in patients undergoing chronic lithium treatment. Prior work has demonstrated differences in physiological effects of the stable lithium isotopes, 6Li and 7Li. Here, we measured the degree of polyuria, polydipsia and kidney histological changes induced in rats by equimolar amounts of 6LiCl, 7LiCl and the commercially available mixture of both isotopes. Rats were given 1.0 mEq/kg of either 6LiCl, 7LiCl or 'nLiCl' (isotope mixture, 93% 7LiCl) by subcutaneous injection twice daily for up to 49 days. Twenty-four-hour urine volume and water intake were measured daily. Kidneys from rats treated for 7 days with 1.5 mEq/kg 6LiCl, 7LiCl and vehicle were examined under light microscopy and histopathologic changes graded on a 4-point scale of severity. All rats showed loss in renal concentrating ability manifested by increasing urine volume and water intake. Peak effects occurred after 9-13 days treatment, then declined to stable levels at two to three times pre-treatment level. Mean peak effect was significantly greater for 6LiCl than for 7LiCl. Chronic effects of 6LiCl (weeks 3-7 of treatment) on polyuria and polydipsia were persistently higher than that of 7LiCl. nLiCl effect was intermediate. Kidneys from rats treated for 7 days with 6LiCl showed more frequently severe lesions in renal tubules than did 7LiCl-treated rats. Our current data and prior studies suggest that elimination or reduction of 6Li from pharmaceutical preparations may merit further evaluation as a possibly less potentially nephrotoxic form of lithium treatment.

  7. Nuclear Science.

    ERIC Educational Resources Information Center

    Pennsylvania State Dept. of Education, Harrisburg. Bureau of Curriculum Services.

    This document is a report on a course in nuclear science for the high school curriculum. The course is designed to provide a basic but comprehensive understanding of the atom in the light of modern knowledge, and to show how people attempt to harness the tremendous energy liberated through fission and fusion reactions. The course crosses what are…

  8. Nuclear Terrorism.

    SciTech Connect

    Hecker, Siegfried S.

    2001-01-01

    As pointed out by several speakers, the level of violence and destruction in terrorist attacks has increased significantly during the past decade. Fortunately, few have involved weapons of mass destruction, and none have achieved mass casualties. The Aum Shinrikyo release of lethal nerve agent, sarin, in the Tokyo subway on March 20, 1995 clearly broke new ground by crossing the threshold in attempting mass casualties with chemical weapons. However, of all weapons of mass destruction, nuclear weapons still represent the most frightening threat to humankind. Nuclear weapons possess an enormous destructive force. The immediacy and scale of destruction are unmatched. In addition to destruction, terrorism also aims to create fear among the public and governments. Here also, nuclear weapons are unmatched. The public's fear of nuclear weapons or, for that matter, of all radioactivity is intense. To some extent, this fear arises from a sense of unlimited vulnerability. That is, radioactivity is seen as unbounded in three dimensions - distance, it is viewed as having unlimited reach; quantity, it is viewed as having deadly consequences in the smallest doses (the public is often told - incorrectly, of course - that one atom of plutonium will kill); and time, if it does not kill you immediately, then it will cause cancer decades hence.

  9. Nuclear medicine

    SciTech Connect

    Wagner, H.N. Jr.

    1986-10-17

    In 1985 and 1986 nuclear medicine became more and more oriented toward in vov chemistry, chiefly as a result of advances in positron emission tomography (PET). The most important trend was the extension of PET technology into the care of patients with brain tumors, epilepsy, and heart disease. A second trend was the increasing use of single-photon emission computed tomography (SPECT).

  10. Nuclear Misinformation

    ERIC Educational Resources Information Center

    Ford, Daniel F.; Kendall, Henry W.

    1975-01-01

    Many scientists feel that research into nuclear safety has been diverted or distorted, and the results of the research concealed or inaccurately reported on a large number of occasions. Of particular concern have been the emergency cooling systems which have not, as yet, been adequately tested. (Author/MA)

  11. Nuclear Science.

    ERIC Educational Resources Information Center

    Pennsylvania State Dept. of Education, Harrisburg. Bureau of Curriculum Services.

    This document is a report on a course in nuclear science for the high school curriculum. The course is designed to provide a basic but comprehensive understanding of the atom in the light of modern knowledge, and to show how people attempt to harness the tremendous energy liberated through fission and fusion reactions. The course crosses what are…

  12. Nuclear orbiting

    SciTech Connect

    Shapira, D.

    1988-01-01

    Nuclear orbiting following collisions between sd and p shell nuclei is discussed. The dependence of this process on the real and imaginary parts of the nucleus-nucleus potential is discussed, as well as the evolution of the dinucleus toward a fully equilibrated fused system. 26 refs., 15 figs.

  13. Nuclear Misinformation

    ERIC Educational Resources Information Center

    Ford, Daniel F.; Kendall, Henry W.

    1975-01-01

    Many scientists feel that research into nuclear safety has been diverted or distorted, and the results of the research concealed or inaccurately reported on a large number of occasions. Of particular concern have been the emergency cooling systems which have not, as yet, been adequately tested. (Author/MA)

  14. Nuclear energy.

    PubMed

    Wilson, Peter D

    2010-01-01

    The technical principles and practices of the civil nuclear industry are described with particular reference to fission and its products, natural and artificial radioactivity elements principally concerned and their relationships, main types of reactor, safety issues, the fuel cycle, waste management, issues related to weapon proliferation, environmental considerations and possible future developments.

  15. NUCLEAR REACTOR

    DOEpatents

    Treshow, M.

    1961-09-01

    A boiling-water nuclear reactor is described wherein control is effected by varying the moderator-to-fuel ratio in the reactor core. This is accomplished by providing control tubes containing a liquid control moderator in the reactor core and providing means for varying the amount of control moderatcr within the control tubes.

  16. Analysis of suprathermal nuclear processes in the solar core plasma

    NASA Astrophysics Data System (ADS)

    Voronchev, Victor T.; Nakao, Yasuyuki; Watanabe, Yukinobu

    2017-04-01

    A consistent model for the description of suprathermal processes in the solar core plasma naturally triggered by fast particles generated in exoergic nuclear reactions is formulated. This model, based on the formalism of in-flight reaction probability, operates with different methods of treating particle slow-down in the plasma, and allows for the influence of electron degeneracy and electron screening on processes in the matter. The model is applied to examine slowing-down of 8.7 MeV α-particles produced in the {}7{Li}(p,α )α reaction of the pp chain, and to analyze suprathermal processes in the solar CNO cycle induced by them. Particular attention is paid to the suprathermal {}14{{N}}{(α ,{{p}})}17{{O}} reaction unappreciated in standard solar model simulations. It is found that an appreciable non-standard (α ,p) nuclear flow due to this reaction appears in the matter and modifies running of the CNO cycle in ∼95% of the solar core region. In this region at R> 0.1{R}ȯ , normal branching of nuclear flow {}14{{N}}≤ftarrow {}17{{O}}\\to {(}18{{F}})\\to {}18{{O}} transforms to abnormal sequential flow {}14{{N}}\\to {}17{{O}}\\to {(}18{{F}})\\to {}18{{O}}, altering some element abundances. In particular, nuclear network calculations reveal that in the outer core the abundances of 17O and 18O isotopes can increase by a factor of 20 as compared with standard estimates. A conjecture is made that other CNO suprathermal (α ,p) reactions may also affect abundances of CNO elements, including those generating solar neutrinos.

  17. Characterization, average and electronic structures during charge-discharge cycle in 0.6Li2MnO3-0.4Li(Co1/3Ni1/3Mn1/3)O2 solid solution of a cathode active material for Li-ion battery

    NASA Astrophysics Data System (ADS)

    Idemoto, Yasushi; Kawai, Ryosuke; Ishida, Naoya; Kitamura, Naoto

    2015-01-01

    The 0.6Li2MnO3-0.4Li(Co1/3Ni1/3Mn1/3)O2 solid solution was prepared by the co-precipitation method. The average structure analysis based on the Rietveld method using neutron diffraction was carried out. As a result, the charging process eliminated Li from the transition metal layer as well as the lithium layer, and the dominant elimination of Li was suggested to be from the 2b site (S.G.; C2/m). The amount of the cation mixing of Ni at the 2c site in the Li layer tended to increase from the first to fifth cycles. It was suggested that Co moved to the 4g site after discharge, but to the 2b site after charging. On the other hand, the opposite tendency was shown for Mn. In addition, an electronic-structure analysis based on the Maximum Entropy Method was carried out. The covalent linkage increased in 4h-4i and 4h-8j between the first and fifth charge processes. It was also found that most of the Li in the 4h site was not extracted at the fifth cycle compared to the first cycle.

  18. Hyperfiltration-induced fractionation of lithium isotopes in geologic systems. Progress report, April 1, 1991--December 1, 1991

    SciTech Connect

    Fritz, S.J.

    1992-01-01

    Effective modeling of hyperfiltration-induced fractionation of lithium isotopes is hindered by a lack of data on aqueous diffusion coefficients of {sup 6}Li{sup +} and {sup 7}Li{sup +}. Several experiments were conducted this past year on yielded a value for the ratio of diffusion coefficients between {sup D6}Li+Cl{minus}/{sup D7}Li+Cl{minus}. A 0.9450 M LiCl solution was placed within sealed dialysis tubing and osmoted against a kilogram of deionized water at 22C. Osmotic equilibrium occurred at 143 minutes, and the ratio of {omega}{sup 6}Li{sup +}Cl{minus}/{omega}{sup 7}Li+Cl{minus} was measured to be 1.011. Because this experimental value is close to the square root of the mass ratio between {sup 7}LiCl and {sup 6}LiCl (1.012), Graham`s Law may be a convenient way to calculate such ratios for aqueous diffusion coefficients of individual isotopic components. In evolution of this closed-system osmotic cell as a function of time, Li isotopic ratios of beaker and bag solutions exhibit a minimum and a maximum before the {sup 6}Li/{sup 7}Li ratios of both solutions assume the inevitable asymptotic approach toward isotopic equilibrium. Max difference in {sup 6}Li/{sup 7}Li ratio between beaker and bag solution was 0.00156 {plus_minus} 0.00015.

  19. Nuclear Medicine

    PubMed Central

    Streek, Penny Vande; Carretta, Robert; Weiland, Frederick L.

    1994-01-01

    The Council on Scientific Affairs of the California Medical Association presents the following epitomes of progress in nuclear medicine. Each item, in the judgment of a panel of knowledgeable physicians, has recently become reasonably firmly established, both as to scientific fact and clinical importance. The items are presented in simple epitome, and an authoritative reference, both to the item itself and to the subject as a whole, is generally given for those who may be unfamiliar with a particular item. The purpose is to assist busy practitioners, students, researchers, and scholars to stay abreast of progress in medicine, whether in their own field of special interest or another. The epitomes included here were selected by the Advisory Panel to the Section on Nuclear Medicine of the California Medical Association, and the summaries were prepared under the direction of Dr Lyons and the panel. PMID:7529452

  20. NUCLEAR REACTOR

    DOEpatents

    Anderson, C.R.

    1962-07-24

    A fluidized bed nuclear reactor and a method of operating such a reactor are described. In the design means are provided for flowing a liquid moderator upwardly through the center of a bed of pellets of a nentron-fissionable material at such a rate as to obtain particulate fluidization while constraining the lower pontion of the bed into a conical shape. A smooth circulation of particles rising in the center and falling at the outside of the bed is thereby established. (AEC)