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Sample records for absolute photoionization cross-sections

  1. Absolute partial photoionization cross sections of ozone.

    SciTech Connect

    Berkowitz, J.; Chemistry

    2008-04-01

    Despite the current concerns about ozone, absolute partial photoionization cross sections for this molecule in the vacuum ultraviolet (valence) region have been unavailable. By eclectic re-evaluation of old/new data and plausible assumptions, such cross sections have been assembled to fill this void.

  2. Absolute Photoionization Cross Sections of Two Cyclic Ketones: Cyclopentanone & Cyclohexanone.

    PubMed

    Price, Chelsea; Fathi, Yasmin; Meloni, Giovanni

    2017-02-23

    Absolute photoionization cross sections for cyclopentanone and cyclohexanone, as well as partial ionization cross sections for the dissociative ionized fragments, are presented in this investigation. Experiments are performed via a multiplexed photoionization mass spectrometer utilizing VUV synchrotron radiation supplied by the Advanced Light Source of Lawrence Berkeley National Laboratory. These results allow the quantification of these species that is relevant to investigate the kinetics and combustion reactions of potential biofuels. The CBS-QB3 calculated values for the adiabatic ionization energies agree well with the experimental values and the identification of possible dissociative fragments is discussed for both systems.

  3. Absolute measurements of chlorine Cl+ cation single photoionization cross section

    NASA Astrophysics Data System (ADS)

    Hernández, E. M.; Juárez, A. M.; Kilcoyne, A. L. D.; Aguilar, A.; Hernández, L.; Antillón, A.; Macaluso, D.; Morales-Mori, A.; González-Magaña, O.; Hanstorp, D.; Covington, A. M.; Davis, V.; Calabrese, D.; Hinojosa, G.

    2015-01-01

    The photoionization of Cl+ leading to Cl2+ was measured in the photon energy range of 19.5-28.0 eV. A spectrum with a photon energy resolution of 15 meV normalized to absolute cross-section measurements is presented. The measurements were carried out by merging a Cl+ ion beam with a photon beam of highly monochromatic synchrotron radiation at the Advanced Light Source at Lawrence Berkeley National Laboratory. The measured photoionization of Cl+ consists of several autoionization resonances surperimposed on the direct photoionization signal. Most of the prominent resonances are assigned to members of Rydberg series originating from the singlet ground state and from metastable triplet levels within the ground-state configuration of Cl+. The direct ionization cross section is no larger than 12 Mb.

  4. Experimental absolute cross section for photoionization of Xe^7+

    NASA Astrophysics Data System (ADS)

    Schippers, S.; Müller, A.; Esteves, D.; Habibi, M.; Aguilar, A.; Kilcoyne, A. L. D.

    2010-03-01

    Collision processes with highly charged xenon ions are of interest for UV-radiation generation in plasma discharges, for fusion research and for space craft propulsion. Here we report results for the photoionization of Xe^7+ ionsootnotetextS. Schippers et al., J. Phys.: Conf. Ser. (in print) which were measured at the photon-ion end station of ALS beamline 10.0.1. As compared with the only previous experimental studyootnotetextJ. M. Bizau et al., Phys. Rev. Lett. 84, 435 (2000) of this reaction, the present cross sections were obtained at higher energy resolution (50--80 meV vs. 200--500 meV) and on an absolute cross section scale. In the experimental photon energy range of 95--145 eV the cross section is dominated by resonances associated with 4d->5f excitation and subsequent autoionization. The most prominent feature in the measured spectrum is the 4d^9,s,f, resonance at 121.14±0.02 eV which reaches a peak cross section of 1.2 Gb at 50 meV photon energy spread. The experimental resonance strength of 160 Mb eV (corresponding to an absorption oscillator strength of 1.46) is in fair agreement with the theoretical result^2.

  5. Absolute single-photoionization cross sections of Se2 +: Experiment and theory

    NASA Astrophysics Data System (ADS)

    Macaluso, D. A.; Aguilar, A.; Kilcoyne, A. L. D.; Red, E. C.; Bilodeau, R. C.; Phaneuf, R. A.; Sterling, N. C.; McLaughlin, B. M.

    2015-12-01

    Absolute single-photoionization cross-section measurements for Se2 + ions were performed at the Advanced Light Source at Lawrence Berkeley National Laboratory using the merged-beams photo-ion technique. Measurements were made at a photon energy resolution of 24 ±3 meV in the photon energy range 23.5-42.5 eV, spanning the ground state and low-lying metastable state ionization thresholds. To clearly resolve the resonant structure near the ground-state threshold, high-resolution measurements were made from 30.0 to 31.9 eV at a photon energy resolution of 6.7 ±0.7 meV. Numerous resonance features observed in the experimental spectra are assigned and their energies and quantum defects tabulated. The high-resolution cross-section measurements are compared with large-scale, state-of-the-art theoretical cross-section calculations obtained from the Dirac Coulomb R -matrix method. Suitable agreement is obtained over the entire photon energy range investigated. These results are an experimental determination of the absolute photoionization cross section of doubly ionized selenium and include a detailed analysis of the photoionization resonance spectrum of this ion.

  6. Near-threshold absolute photoionization cross-sections of some reaction intermediates in combustion

    NASA Astrophysics Data System (ADS)

    Wang, Juan; Yang, Bin; Cool, Terrill A.; Hansen, Nils; Kasper, Tina

    2008-02-01

    The use of photoionization mass spectrometry for the development of quantitative kinetic models for the complex combustion chemistry of both conventional hydrocarbon fuels and oxygenated biofuels requires near-threshold measurements of absolute photoionization cross-sections for numerous reaction intermediates. Near-threshold absolute cross-sections for molecular and dissociative photoionization for 20 stable reaction intermediates (methane, ethane, propane, n-butane, cyclopropane, methylcyclopentane, 1-butene, cis-2-butene, isobutene, 1-pentene, cyclohexene, 3,3-dimethyl-1-butene, 1,3-hexadiene, 1,3-cyclohexadiene, methyl acetate, ethyl acetate, tetrahydrofuran, propanal, 1-butyne, 2-butyne) are presented. Previously measured total photoionization cross-sections for 9 of these molecules are in good agreement with the present results. The measurements are performed with photoionization mass spectrometry (PIMS) using a monochromated VUV synchrotron light source with an energy resolution of 40 meV (fwhm) comparable to that used for flame-sampling molecular beam PIMS studies of flame chemistry and reaction kinetics.

  7. Absolute photoionization cross sections of furanic fuels: 2-ethylfuran, 2-acetylfuran and furfural.

    PubMed

    Smith, Audrey R; Meloni, Giovanni

    2015-11-01

    Absolute photoionization cross sections of the molecules 2-ethylfuran, 2-acetylfuran and furfural, including partial ionization cross sections for the dissociative ionized fragments, are measured for the first time. These measurements are important because they allow fuel quantification via photoionization mass spectrometry and the development of quantitative kinetic modeling for the complex combustion of potential fuels. The experiments are carried out using synchrotron photoionization mass spectrometry with an orthogonal time-of-flight spectrometer used for mass analysis at the Advanced Light Source of Lawrence Berkeley National Laboratory. The CBS-QB3 calculations of adiabatic ionization energies and appearance energies agree well with the experimental results. Several bond dissociation energies are also derived and presented.

  8. Absolute single photoionization cross-section measurements of Rb2+ ions: experiment and theory

    NASA Astrophysics Data System (ADS)

    Macaluso, D. A.; Bogolub, K.; Johnson, A.; Aguilar, A.; Kilcoyne, A. L. D.; Bilodeau, R. C.; Bautista, M.; Kerlin, A. B.; Sterling, N. C.

    2016-12-01

    Absolute single photoionization cross-section measurements of Rb2+ ions were performed using synchrotron radiation and the photo-ion, merged-beams technique at the Advanced Light Source at Lawrence Berkeley National Laboratory. Measurements were made at a photon energy resolution of 13.5 ± 2.5 meV from 37.31 to 44.08 eV spanning the 2P{}3/2o ground state and 2P{}1/2o metastable state ionization thresholds. Multiple autoionizing resonance series arising from each initial state are identified using quantum defect theory. The measurements are compared to Breit-Pauli R-matrix calculations with excellent agreement between theory and experiment.

  9. Absolute Total Photoionization Cross Section of C60 in the Range of 25-120 eV: Revisited

    NASA Astrophysics Data System (ADS)

    Kafle, Bhim P.; Katayanagi, Hideki; Prodhan, Md. Serajul I.; Yagi, Hajime; Huang, Chaoqun; Mitsuke, Koichiro

    2008-01-01

    The absolute total photoionization cross section σabs,I of gaseous C60 is measured in the photon energy hν range from 25 to 120 eV by photoionization mass spectrometry with synchrotron radiation. The absolute detection efficiencies of photoions in different charge states are evaluated. The present σabs,I curve is combined with the photoabsorption cross section curves of C60 at hν=3.5--26 eV in the literature, after appropriate alterations of the vapor pressure are taken into account. The oscillator strengths are computed from the composite curve to be 178.5 and 230.5 for the hν ranges from 3.5 to 40.8 eV and from 3.5 to 119 eV, respectively. These oscillator strengths agree well with those expected from the Thomas-Kuhn-Reiche sum rule and 60 times the photoabsorption cross section of a carbon atom. Moreover, the present σabs,I curve behaves similarly to the relative photoionization cross section curve reported by Reinköster et al.

  10. Photoionization of Ne Atoms and Ne+ Ions Near the K Edge: Precision Spectroscopy and Absolute Cross-sections

    NASA Astrophysics Data System (ADS)

    Müller, Alfred; Bernhardt, Dietrich; Borovik, Alexander, Jr.; Buhr, Ticia; Hellhund, Jonas; Holste, Kristof; Kilcoyne, A. L. David; Klumpp, Stephan; Martins, Michael; Ricz, Sandor; Seltmann, Jörn; Viefhaus, Jens; Schippers, Stefan

    2017-02-01

    Single, double, and triple photoionization of Ne+ ions by single photons have been investigated at the synchrotron radiation source PETRA III in Hamburg, Germany. Absolute cross-sections were measured by employing the photon-ion merged-beams technique. Photon energies were between about 840 and 930 eV, covering the range from the lowest-energy resonances associated with the excitation of one single K-shell electron up to double excitations involving one K- and one L-shell electron, well beyond the K-shell ionization threshold. Also, photoionization of neutral Ne was investigated just below the K edge. The chosen photon energy bandwidths were between 32 and 500 meV, facilitating the determination of natural line widths. The uncertainty of the energy scale is estimated to be 0.2 eV. For comparison with existing theoretical calculations, astrophysically relevant photoabsorption cross-sections were inferred by summing the measured partial ionization channels. Discussion of the observed resonances in the different final ionization channels reveals the presence of complex Auger-decay mechanisms. The ejection of three electrons from the lowest K-shell-excited Ne+(1s2{s}22{p}6{}2{{{S}}}1/2) level, for example, requires cooperative interaction of at least four electrons.

  11. Photoionization of Ne Atoms and Ne + Ions Near the K Edge: PrecisionSpectroscopy and Absolute Cross-sections

    DOE PAGES

    Müller, Alfred; Bernhardt, Dietrich; Borovik, Alexander; ...

    2017-02-17

    Single, double, and triple photoionization of Ne + ions by single photons have been investigated at the synchrotron radiation source PETRA III in Hamburg, Germany. Absolute cross-sections were measured by employing the photon-ion merged-beams technique. Photon energies were between about 840 and 930 eV, covering the range from the lowest-energy resonances associated with the excitation of one single K-shell electron up to double excitations involving one K- and one L-shell electron, well beyond the K-shell ionization threshold. Also, photoionization of neutral Ne was investigated just below the K edge. The chosen photon energy bandwidths were between 32 and 500 meV,more » facilitating the determination of natural line widths. The uncertainty of the energy scale is estimated to be 0.2 eV. For comparison with existing theoretical calculations, astrophysically relevant photoabsorption cross-sections were inferred by summing the measured partial ionization channels. Discussion of the observed resonances in the different final ionization channels reveals the presence of complex Auger-decay mechanisms. The ejection of three electrons from the lowest K-shell-excited Ne + (1s2s2p6 2S1/2) level, for example, requires cooperative interaction of at least four electrons.« less

  12. Absolute measurement of the photoionization cross section of atomic hydrogen with a shock tube for the extreme ultraviolet. [for astrophysical applications

    NASA Technical Reports Server (NTRS)

    Palenius, H. P.; Kohl, J. L.; Parkinson, W. H.

    1976-01-01

    The paper reports an experiment which is part of a program to measure the absolute values of the atomic photoionization cross sections of astrophysically abundant elements, particularly in stars and planetary atmospheres. An aerodynamic pressure-driven shock tube constructed from stainless steel with a quadratic cross section was used to measure the photoionization cross section of H I at 19 wavelength points from 910 to 609 A with experimental uncertainties between 7 and 20%. The shock tube was used to produce fully dissociated hydrogen and neon mixtures for the photoabsorption measurements.

  13. Absolute measurements of photoabsorption, Photoionization, and photodissociation cross sections of SiH4 and Si2H6 in the 13-22 eV region

    NASA Astrophysics Data System (ADS)

    Kameta, Kosei; Ukai, Masatoshi; Terazawa, Norihisa; Nagano, Kazunori; Chikahiro, Yuji; Kouchi, Norihuki; Hatano, Yoshihiko; Tanaka, Kenichiro

    1992-07-01

    The absolute values of the photoabsorption cross sections and photoionization quantum yields of silane and disilane have been measured in the 13-22 eV region. Using these values, we have evaluated the absolute cross sections of the photoionization and neutral dissociation. The individual structures observed in the cross section spectra have been interpreted in terms of the characters of superexcited states with strong emphasis on the neutral dissociation. The 3a1-1σ*(t2) state of silane presenting a broad peak at around 14.6 eV in an absorption cross section is shown to be strongly dissociative, whereas Rydberg series to the (3a1)-1 limit showing up vibrational structures between 16 and 18 eV predominantly undergo fast autoionization decay. A general importance of competition between autoionization and neutral dissociation is indicated of disilane in much higher energy region than the first ionization potential.

  14. Determination of the absolute photoionization cross sections of CH3 and I produced from a pyrolysis source, by combined synchrotron and vacuum ultraviolet laser studies.

    PubMed

    Gans, Bérenger; Vieira Mendes, Luiz A; Boyé-Péronne, Séverine; Douin, Stéphane; Garcia, Gustavo; Soldi-Lose, Héloïse; Cunha de Miranda, Barbara K; Alcaraz, Christian; Carrasco, Nathalie; Pernot, Pascal; Gauyacq, Dolores

    2010-03-11

    A pyrolysis source coupled to a supersonic expansion has been used to produce the CH3 radical from two precursors, iodomethane CH3I and nitromethane CH3NO2. The relative ionization yield of CH3 has been recorded at the SOLEIL Synchrotron Radiation source in the range 9.0-11.6 eV, and its ionization threshold has been modeled by taking into account the vibrational and rotational temperature of the radical in the molecular beam. The relative photoionization yield has been normalized to an absolute cross section scale at a fixed wavelength (118.2 nm, sigma(i)(CH3) = 6.7(-1.8)(+2.4) Mb, 95% confidence interval) in an independent laboratory experiment using the same pyrolysis source, a vacuum ultraviolet (VUV) laser, and a carefully calibrated detection chain. The resulting absolute cross section curve is in good agreement with the recently published measurements by Taatjes et al., although with an improved signal-to-noise ratio. The absolute photoionization cross section of CH3I at 118.2 nm has also been measured to be sigma(i)(CH3I) = (48.2 +/- 7.9) Mb, in good agreement with previous electron impact measurements. Finally, the photoionization yield of the iodine atom in its ground state 2P(3/2) has been recorded using the synchrotron source and calibrated for the first time on an absolute cross section scale from our fixed 118.2 nm laser measurement, sigma(i)(I2P(3/2)) = 74(-23)(+33) Mb (95% confidence interval). The ionization curve of atomic iodine is in good agreement, although with slight variations, with the earlier relative ionization yield measured by Berkowitz et al. and is also compared to an earlier calculation of the iodine cross section by Robicheaux and Greene. It is demonstrated that, in the range of pyrolysis temperature used in this work, all the ionization cross sections are temperature-independent. Systematic care has been taken to include all uncertainty sources contributing to the final confidence intervals for the reported results.

  15. Determining the partial photoionization cross-sections of ethyl radicals.

    PubMed

    FitzPatrick, B L; Maienschein-Cline, M; Butler, L J; Lee, S-H; Lin, J J

    2007-12-13

    Using a crossed laser-molecular beam scattering apparatus, these experiments photodissociate ethyl chloride at 193 nm and detect the Cl and ethyl products, resolved by their center-of-mass recoil velocities, with vacuum ultraviolet photoionization. The data determine the relative partial cross-sections for the photoionization of ethyl radicals to form C2H5+, C2H4+, and C2H3+ at 12.1 and 13.8 eV. The data also determine the internal energy distribution of the ethyl radical prior to photoionization, so we can assess the internal energy dependence of the photoionization cross-sections. The results show that the C2H4++H and C2H3++H2 dissociative photoionization cross-sections strongly depend on the photoionization energy. Calibrating the ethyl radical partial photoionization cross-sections relative to the bandwidth-averaged photoionization cross-section of Cl atoms near 13.8 eV allows us to use these data in conjunction with literature estimates of the Cl atom photoionization cross-sections to put the present bandwidth-averaged cross-sections on an absolute scale. The resulting bandwidth-averaged cross-section for the photoionization of ethyl radicals to C2H5+ near 13.8 eV is 8+/-2 Mb. Comparison of our 12.1 eV data with high-resolution ethyl radical photoionization spectra allows us to roughly put the high-resolution spectrum on the same absolute scale. Thus, one obtains the photoionization cross-section of ethyl radicals to C2H5+ from threshold to 12.1 eV. The data show that the onset of the C2H4++H dissociative photoionization channel is above 12.1 eV; this result offers a simple way to determine whether the signal observed in photoionization experiments on complex mixtures is due to ethyl radicals. We discuss an application of the results for resolving the product branching in the O+allyl bimolecular reaction.

  16. K-shell photoionization cross-sections.

    NASA Technical Reports Server (NTRS)

    Daltabuit, E.; Cox, D. P.

    1972-01-01

    Approximate values for the threshold energies, threshold cross sections, and energy dependence of the cross sections for K-shell photoionization are tabulated for H, He, C, N, O, Ne, Mg, Si, and S in all stages of ionization. The approximation of these data is based on the assumptions that the threshold energy is a simple function of the nuclear charge and the number of electrons present in the atom, and that the threshold values and energy dependence of the cross sections are determined only by the threshold energy.

  17. Photodissociation of Acetaldehyde and the Photoionization Cross Section of HCO

    NASA Astrophysics Data System (ADS)

    Shubert, V. Alvin; Pratt, Stephen T.

    2010-06-01

    Acetaldehyde was photodissociated with near UV laser light, and the methyl (CH_3) and formyl (HCO) radical fragments were photoionized with vacuum ultraviolet (VUV) light. The fragments were detected by using both time of flight mass spectrometry and velocity ion map imaging. With the former technique, simultaneous detection of both fragments provided the intensity of HCO+ relative to CH_3+ with I(HCO+)/I(CH_3+) ≈ 0.8. Because the absolute photoionization cross section of the CH_3 radical has been characterized (≈ 5 Mb) at the VUV energies of interest, the absolute photoionization cross section of HCO could be determined from the intensity ratio, yielding an HCO cross section of ≈ 4 Mb at 10.3 eV. However, because some of the HCO fragments could be formed with enough internal energy to undergo secondary dissociation, velocity ion map imaging was employed to determine the extent of any secondary dissociation that occurred. The translational energy distributions obtained for both the CH_3 and HCO fragments are nearly identical, indicating that no HCO fragments underwent secondary dissociation. A surprising result was the smaller photoionization cross section of HCO relative to CH_3. Comparison to the isoelectronic species of NO will be discussed and a potential explanation will be offered for this observation. This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under contract No. DE-AC02-06CH11357.

  18. Absolute cross sections of compound nucleus reactions

    NASA Astrophysics Data System (ADS)

    Capurro, O. A.

    1993-11-01

    The program SEEF is a Fortran IV computer code for the extraction of absolute cross sections of compound nucleus reactions. When the evaporation residue is fed by its parents, only cumulative cross sections will be obtained from off-line gamma ray measurements. But, if one has the parent excitation function (experimental or calculated), this code will make it possible to determine absolute cross sections of any exit channel.

  19. Photoionization research on atomic beams. 2: The photoionization cross section of atomic oxygen

    NASA Technical Reports Server (NTRS)

    Comes, F. J.; Speier, F.; Elzer, A.

    1982-01-01

    An experiment to determine the absolute value of the photo-ionization cross section of atomic oxygen is described. The atoms are produced in an electrical discharge in oxygen gas with 1% hydrogen added. In order to prevent recombination a crossed beam technique is employed. The ions formed are detected by a time-of-flight mass spectrometer. The concentration of oxygen atoms in the beam is 57%. The measured photoionization cross section of atomic oxygen is compared with theoretical data. The results show the participation of autoionization processes in ionization. The cross section at the autoionizing levels detected is considerably higher than the absorption due to the unperturbed continuum. Except for wavelengths where autoionization occurs, the measured ionization cross section is in fair agreement with theory. This holds up to 550 A whereas for shorter wavelengths the theoretical values are much higher.

  20. VUV photoionization cross sections of HO2, H2O2, and H2CO.

    PubMed

    Dodson, Leah G; Shen, Linhan; Savee, John D; Eddingsaas, Nathan C; Welz, Oliver; Taatjes, Craig A; Osborn, David L; Sander, Stanley P; Okumura, Mitchio

    2015-02-26

    The absolute vacuum ultraviolet (VUV) photoionization spectra of the hydroperoxyl radical (HO2), hydrogen peroxide (H2O2), and formaldehyde (H2CO) have been measured from their first ionization thresholds to 12.008 eV. HO2, H2O2, and H2CO were generated from the oxidation of methanol initiated by pulsed-laser-photolysis of Cl2 in a low-pressure slow flow reactor. Reactants, intermediates, and products were detected by time-resolved multiplexed synchrotron photoionization mass spectrometry. Absolute concentrations were obtained from the time-dependent photoion signals by modeling the kinetics of the methanol oxidation chemistry. Photoionization cross sections were determined at several photon energies relative to the cross section of methanol, which was in turn determined relative to that of propene. These measurements were used to place relative photoionization spectra of HO2, H2O2, and H2CO on an absolute scale, resulting in absolute photoionization spectra.

  1. Photoabsorption and photoionization cross sections for formaldehyde in the vacuum-ultraviolet energy range

    NASA Astrophysics Data System (ADS)

    Tanaka, H. K.; Prudente, F. V.; Medina, A.; Marinho, R. R. T.; Homem, M. G. P.; Machado, L. E.; Fujimoto, M. M.

    2017-03-01

    We report a theoretical-experimental investigation on the interaction of vacuum-ultraviolet radiation with formaldehyde (H2CO) in the gas phase. Experimentally, the absolute photoabsorption cross sections and the photoionization quantum yields were measured in the (11.0-21.5) eV range using the double-ion chamber technique. Also, the absolute photoionization and neutral-decay cross sections were derived from these data. In addition, in the same energy region, the dissociation pattern was obtained with a time-of-flight mass spectrometer using the photoelectron-photoion coincidence technique, and the absolute photoionization cross sections were derived for each ionic fragment observed. Moreover, theoretical photoionization cross sections were calculated for the ionization of the four outermost molecular valence orbitals (2b2, 1b1, 5a1, and 1b2) from the threshold to 35 eV. The calculations were performed using the iterative Schwinger variational method to solve the Lippmann-Schwinger equation in the exact static-exchange level of approximation. In general, there is a good agreement between our experimental and previous data reported in the literature. Our theoretical results show a fair qualitative agreement with the experimental data and with previous theoretical results. Above 20 eV, a better quantitative agreement with the experimental data is also observed.

  2. Vibrationally resolved C 1s photoionization cross section of CF4

    NASA Astrophysics Data System (ADS)

    Patanen, M.; Kooser, K.; Argenti, L.; Ayuso, D.; Kimura, M.; Mondal, S.; Plésiat, E.; Palacios, A.; Sakai, K.; Travnikova, O.; Decleva, P.; Kukk, E.; Miron, C.; Ueda, K.; Martín, F.

    2014-06-01

    The differential photoionization cross section ratio (ν = 1)/(ν = 0) for the symmetric stretching mode in the C 1s photoionization of CF4 was studied both theoretically and experimentally. We observed this ratio to differ from the Franck-Condon ratio and to be strongly dependent on the photon energy, even far from the photoionization threshold. The density-functional theory computations show that the ratio is significantly modulated by the diffraction of the photoelectrons by the neighbouring atoms at high photon energies. At lower energies, the interpretation of the first very strong maximum observed about 60 eV above the photoionization threshold required detailed calculations of the absolute partial cross sections, which revealed that the absolute cross section has two maxima at lower energies, which turn into one maximum in the cross section ratio because the maxima appear at slightly different energies in ν = 1 and ν = 0 cross sections. These two strong, low-energy continuum resonances originate from the trapping of the continuum wavefunction in the molecular potential of the surrounding fluorine atoms and from the outgoing electron scattering by them.

  3. Total and dissociative photoionization cross sections of N2 from threshold to 107 eV

    NASA Technical Reports Server (NTRS)

    Samson, James A. R.; Masuoka, T.; Pareek, P. N.; Angel, G. C.

    1986-01-01

    The absolute cross sections for the production of N(+) and N2(+) were measured from the dissociative ionization threshold of 115 A. In addition, the absolute photoabsorption and photoionization cross sections were tabulated between 114 and 796 A. The ionization efficiencies were also given at several discrete wave lengths between 660 and 790 A. The production of N(+) fragment ions are discussed in terms of the doubly excited N2(+) states with binding energies in the range of 24 to 44 eV.

  4. Intermanifold similarities in partial photoionization cross sections of helium

    NASA Astrophysics Data System (ADS)

    Schneider, Tobias; Liu, Chien-Nan; Rost, Jan-Michael

    2002-04-01

    Using the eigenchannel R-matrix method we calculate partial photoionization cross sections from the ground state of the helium atom for incident photon energies up to the N=9 manifold. The wide energy range covered by our calculations permits a thorough investigation of general patterns in the cross sections which were first discussed by Menzel and coworkers [Phys. Rev. A 54, 2080 (1996)]. The existence of these patterns can easily be understood in terms of propensity rules for autoionization. As the photon energy is increased the regular patterns are locally interrupted by perturber states until they fade out indicating the progressive breakdown of the propensity rules and the underlying approximate quantum numbers. We demonstrate that the destructive influence of isolated perturbers can be compensated with an energy-dependent quantum defect.

  5. Differential cross section for the double photoionization of Mg

    NASA Astrophysics Data System (ADS)

    Abdel-Naby, Shahin A.; Pindzola, M. S.; Colgan, J.

    2015-01-01

    The time-dependent close-coupling (TDCC) method is used to calculate the energy and angle triple differential cross section for the double photoionization of Mg(3{{s}2}) at a photon energy of 55.49 eV to compare with recent converged close-coupling (CCC) calculations and in support of recent experiments at ELETTRA. Comparisons are made between the TDCC, CCC, and experimental results for equal energy sharing at scattering angles of 0{}^\\circ , 30{}^\\circ , and 60{}^\\circ , and for unequal energy sharing at 0{}^\\circ and 30{}^\\circ . Comparisons are made between the TDCC and CCC results for equal and unequal energy sharing at 90{}^\\circ . In addition, TDCC, CCC, and experimental results are compared for complex scattering amplitudes and the TDCC method is used to calculate single energy differential cross sections at photon energies of 30, 35, 40, 45, and 55.49 eV. Although there are scattering angles in the triple differential cross sections at 55.49 eV at which the TDCC, CCC, and experimental results are quite different, the overall agreement between the theories and experiment is reasonable for such small cross sections.

  6. Photoionization cross section measurements of the excited states of cobalt in the near-threshold region

    SciTech Connect

    Zheng, Xianfeng Zhou, Xiaoyu; Cheng, Zaiqi; Jia, Dandan; Qu, Zehua; Yao, Guanxin; Zhang, Xianyi; Cui, Zhifeng

    2014-10-15

    We present measurements of photoionization cross-sections of the excited states of cobalt using a two-color, two-step resonance ionization technique in conjunction with a molecular beam time of flight (TOF) mass spectrometer. The atoms were produced by the laser vaporization of a cobalt rod, coupled with a supersonic gas jet. The absolute photoionization cross-sections at threshold and near-threshold regions (0-1.2 eV) were measured, and the measured values ranged from 4.2±0.7 Mb to 10.5±1.8 Mb. The lifetimes of four odd parity energy levels are reported for the first time.

  7. Absolute photoneutron cross sections of Sm isotopes

    SciTech Connect

    Gheorghe, I.; Glodariu, T.; Utsunomiya, H.; Filipescu, D.; Nyhus, H.-T.; Renstrom, T.; Tesileanu, O.; Shima, T.; Takahisa, K.; Miyamoto, S.

    2015-02-24

    Photoneutron cross sections for seven samarium isotopes, {sup 144}Sm, {sup 147}Sm, {sup 148}Sm, {sup 149}Sm, {sup 150}Sm, {sup 152}Sm and {sup 154}Sm, have been investigated near neutron emission threshold using quasimonochromatic laser-Compton scattering γ-rays produced at the synchrotron radiation facility NewSUBARU. The results are important for nuclear astrophysics calculations and also for probing γ-ray strength functions in the vicinity of neutron threshold. Here we describe the neutron detection system and we discuss the related data analysis and the necessary method improvements for adapting the current experimental method to the working parameters of the future Gamma Beam System of Extreme Light Infrastructure - Nuclear Physics facility.

  8. Effect of strongly coupled plasma on photoionization cross section

    SciTech Connect

    Das, Madhusmita

    2014-01-15

    The effect of strongly coupled plasma on the ground state photoionization cross section is studied. In the non relativistic dipole approximation, cross section is evaluated from bound-free transition matrix element. The bound and free state wave functions are obtained by solving the radial Schrodinger equation with appropriate plasma potential. We have used ion sphere potential (ISP) to incorporate the plasma effects in atomic structure calculation. This potential includes the effect of static plasma screening on nuclear charge as well as the effect of confinement due to the neighbouring ions. With ISP, the radial equation is solved using Shooting method approach for hydrogen like ions (Li{sup +2}, C{sup +5}, Al{sup +12}) and lithium like ions (C{sup +3}, O{sup +5}). The effect of strong screening and confinement is manifested as confinement resonances near the ionization threshold for both kinds of ions. The confinement resonances are very much dependent on the edge of the confining potential and die out as the plasma density is increased. Plasma effect also results in appearance of Cooper minimum in lithium like ions, which was not present in case of free lithium like ions. With increasing density the position of Cooper minimum shifts towards higher photoelectron energy. The same behaviour is also true for weakly coupled plasma where plasma effect is modelled by Debye-Huckel potential.

  9. Vibrationally resolved cross sections for the photoionization of CS2

    NASA Astrophysics Data System (ADS)

    Stratmann, R. E.; Lucchese, Robert R.

    1994-12-01

    We have performed vibrationally resolved calculations of the excitation of the symmetric stretch in the photoionization of CS2 leading to the X 2Πg, A 2Πu, B 2Σ+u, and C 2Σ+g states of CS+2. Previous theoretical work has determined that the kπg shape resonance in the (5σu)-1 channel consists mainly of a linear combination of low lying virtual d orbitals on sulfur and is thus essentially atomic in nature. This conclusion was primarily based on the shape of the resonant wave function and the insensitivity of the energy of the resonance to bond stretching. Here, we have determined that the energies of the kπ shape resonances located well above threshold and the σ bound states just below threshold are insensitive to bond length. We have also found nearly constant vibrational branching ratios in all channels and polarization components. This is in qualitative agreement with experimental vibrationally resolved cross sections [S. Kakar, H. C. Choi, and E. D. Poliakoff, J. Chem. Phys. 97, 4690 (1992)] which show nearly constant vibrational branching ratios. Our present results indicate that caution must be exercised when using bond length sensitivity as an exclusive means to determine the existence of shape resonances.

  10. Photoionization and photoabsorption cross sections for the aluminum iso-nuclear sequence

    SciTech Connect

    Witthoeft, M.C.; García, J.; Kallman, T.R.; Palmeri, P.; Quinet, P.

    2013-01-15

    K-shell photoionization and photoabsorption cross sections are presented for Li-like to Na-like Al. The calculations are performed using the Breit–Pauli R-matrix method where the effects of radiation and Auger dampings are included. We provide electronic data files for the raw cross sections as well as those convolved with a Gaussian of width ΔE/E=10{sup −4}. In addition to total cross sections for photoabsorption and photoionization, partial cross sections are available for photoionization.

  11. Total photoionization cross sections of atomic oxygen from threshold to 44.3A

    NASA Technical Reports Server (NTRS)

    Angel, G. C.; Samson, James A. R.

    1987-01-01

    The relative cross section of atomic oxygen for the production of singly charged ions has been remeasured in more detail and extended to cover the wavelength range 44.3 to 910.5 A by the use of synchrotron radiation. In addition, the contribution of multiple ionization to the cross sections has been measured allowing total photoionization cross sections to be obtained below 250 A. The results have been made absolute by normalization to previously measured data. The use of synchrotron radiation has enabled measurements of the continuum cross section to be made between the numerous autoionizing resonances that occur near the ionization thresholds. This in turn has allowed a more critical comparison of the various theoretical estimates of the cross section to be made. The series of autoionizing resonances leading to the 4-P state of the oxygen ion have been observed for the first time in an ionization type experiment and their positions compared with both theory and previous photographic recordings.

  12. Photoionization cross sections of the excited 3s3p 3Po state for atomic Mg

    NASA Astrophysics Data System (ADS)

    Wang, Guoli; Wan, Jianjie; Zhou, Xiaoxin

    2017-01-01

    The photoionization cross sections of the excited levels (3s3p 0,1,2,o 3P) of atomic Mg have been studied theoretically using both the nonrelativistic and fully relativistic R-matrix method. For the threshold cross sections, as previous nonrelativistic studies, present calculations show significant differences (a factor of 3) from former experimental values. Large discrepancies with experiment calls for additional measurements of the photoionization cross sections from the excited states of Mg.

  13. TDLDA calculations of photoionization cross-section and asymmetry parameter profiles of alkaline-earth atoms

    NASA Astrophysics Data System (ADS)

    Stener, M.; De Alti, G.; Fronzoni, G.; Decleva, P.

    1997-10-01

    Absolute photoionization cross-section and asymmetry parameter profiles of Be, Mg and Ca have been calculated at TDLDA and LDA level, employing a very accurate B-spline basis set and the modified Sternheimer approach. The van Leeuwen-Baerends (VLB) exchange correlation potential has been used, since its correct asymptotic behaviour is able to support virtual states and to describe core-excited resonances. The results have been compared with other calculations and experiment when available. The autoionization resonances have been successfully fitted with a suitable Fano profile. The Ca 3p → 3d 'giant-resonance' has been properly described, despite of the dramatic screening effects involved in the process. The success of the TDLDA method for describing the cross-section profiles in the present systems which display a wide range of many-body effects, seems to suggest that further efforts to apply the present method to molecules are justified.

  14. Vacuum ultraviolet photoionization mass spectra and cross-sections for volatile organic compounds at 10.5 eV.

    PubMed

    Kanno, Nozomu; Tonokura, Kenichi

    2007-08-01

    Vacuum ultraviolet single-photon ionization time-of-flight mass spectrometry (VUV-SPI-TOFMS) has been applied to the detection of volatile organic compounds (VOCs), including aromatic, chlorinated, and oxygenated compounds. Photoionization mass spectra of 23 VOCs were measured using SPI-TOFMS at 10.5 eV (118 nm). The limits of detection of VOCs using SPI-TOFMS at 10.5 eV were estimated to be a few ppbv. The mass spectra of 20 VOCs exhibit only the parent ion and its isotopes' signals. The ionization processes of the VOCs were discussed on the basis of the reaction enthalpies predicted by the quantum chemical calculations. Absolute photoionization cross-sections for 23 VOCs, including 12 newly measured VOCs, at 10.5 eV were determined in comparison to the reported absolute photoionization cross-section of NO.

  15. 242Pu absolute neutron-capture cross section measurement

    NASA Astrophysics Data System (ADS)

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; Bucher, B.; Chyzh, A.; Bredeweg, T. A.; Baramsai, B.; Couture, A.; Jandel, M.; Mosby, S.; O'Donnell, J. M.; Ullmann, J. L.

    2017-09-01

    The absolute neutron-capture cross section of 242Pu was measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. During target fabrication, a small amount of 239Pu was added to the active target so that the absolute scale of the 242Pu(n,γ) cross section could be set according to the known 239Pu(n,f) resonance at En,R = 7.83 eV. The relative scale of the 242Pu(n,γ) cross section covers four orders of magnitude for incident neutron energies from thermal to ≈ 40 keV. The cross section reported in ENDF/B-VII.1 for the 242Pu(n,γ) En,R = 2.68 eV resonance was found to be 2.4% lower than the new absolute 242Pu(n,γ) cross section.

  16. Calculated photoionization cross sections using Quantemol-N

    NASA Astrophysics Data System (ADS)

    Brigg, Will J.; Harvey, Alex G.; Dzarasova, Anna; Mohr, Sebastian; Brambila, Danilo S.; Morales, Felipe; Smirnova, Olga; Tennyson, Jonathan

    2015-06-01

    Quantemol-N is an expert system designed to run the widely used UK Molecular R-matrix code (UKRMol). Originally designed to consider electron-molecule collision problems, here we present an extension to treat molecular photoionization. Sample results are given for the photoionization of molecular nitrogen and methane. Comparisons are made with experimental results showing good agreement.

  17. Converged cross-section results for double photoionization of helium atoms in hyperspherical partial wave theory at 6 eV above threshold

    SciTech Connect

    Das, J.N.; Paul, S.; Chakrabarti, K.

    2004-04-01

    Here we report a set of converged cross-section results for double photoionization of helium atoms obtained in the hyperspherical partial wave theory for equal energy sharing kinematics at 6 eV energy above threshold. The calculated cross section results are generally in excellent agreement with the absolute measured results of Doerner et al. [Phys. Rev. 57, 1074 (1998)].

  18. Cross sections for photoionization of fullerene molecular ions C n + with n = 40, 50, 70, 76, 78, and 84

    NASA Astrophysics Data System (ADS)

    Thomas, C. M.; Baral, K. K.; Aryal, N. B.; Habibi, M.; Esteves-Macaluso, D. A.; Kilcoyne, A. L. D.; Aguilar, A.; Schlachter, A. S.; Schippers, S.; Müller, A.; Phaneuf, R. A.

    2017-05-01

    Absolute cross-section measurements are reported for single photoionization of C n + fullerene molecular ions (n =40 , 50, 70, 76, 78, and 84) in the photon-energy range 18-70 eV. The experiments were performed by merging a mass and charge selected beam of C n + molecular ions with a beam of monochromatized synchrotron radiation and measuring the yield of C n 2 + product ions as a function of the photon energy. Oscillator strengths determined by integrating the measured cross sections over this energy range exhibit a linear dependence on n . The cross sections are parametrized by fits to three Lorentzian functions to represent plasmon excitations and a linear function for direct ionization. The highest-energy resonance in the data near 46 eV is similar to that previously observed in single photoionization of C60 and may be attributable to a harmonic of the dominant surface-plasmon resonance near 23 eV.

  19. Partial and total cross sections and multiplet structure in the photoionization of atomic manganese

    SciTech Connect

    Jimenez-Mier, J.; Krause, M.O.; Gerard, P. ); Hermsmeier, B.; Fadley, C.S.

    1989-10-01

    We determined the absolute partial photoionization cross section {sigma} and the angular distribution parameter {beta} of the 3{ital d}, 3{ital p}, and 3{ital s} photoelectrons in atomic manganese for 65{le}{ital h}{nu}{le}250 eV. The total photoionization cross section is in satisfactory accord with the single-particle Hartree-Slater calculation and in very good agreement with a relativistic time-dependent local-density-approximation calculation. Binding energies and intensity ratios of the 3{ital s}{sup {minus}1} and 3{ital p}{sup {minus}1} multiplet lines were obtained. Five lines were identified within the 3{ital p}{sup {minus}1} multiplet, and the measured spacings are close to those found in solid MnF{sub 2}. Similarly, the spacings in the 3{ital s}{sup {minus}1} multiplet are equal to the ones measured in solid MnF{sub 2}. There is good accord between our results for the angular-distribution parameter of the 3{ital p}{sup {minus}1} ({sup 7}P) line and those of Malutzki {ital et} {ital al}. (J. Phys. B 18, 1735 (1985)). The intensity ratios of {sup 5}P(1) to {sup 7}P and {sup 5}S(1) to {sup 7}S were seen to increase slowly somewhat above their thresholds. More rapid variations of all multiplet ratios were found within about 30 eV of threshold.

  20. Relative partial cross sections for single, double, and triple photoionization of C60 and C70.

    PubMed

    Mitsuke, Koichiro; Katayanagi, Hideki; Kafle, Bhim P; Huang, Chaoqun; Yagi, Hajime; Prodhan, Md Serajul I; Kubozono, Yoshihiro

    2007-08-30

    Partial cross sections for the photoion formation from C(60) and C(70) were determined from the yields of singly, doubly, and triply charged ions which were measured by mass spectrometry combined with tunable synchrotron radiation at hnu = 25-120 eV. The dependence of the detection efficiencies on the mass-to-charge ratio was evaluated by using the formula proposed by Twerenbold et al. Corrections of the detection efficiency were found to be critical for obtaining accurate partial cross sections for photoionization of fullerenes. Revisions were made of the partial cross-section curves for single and double photoionization of C(60) and C(70). The curve for triple photoionization of C(70) was newly proposed. The ratios between the cross sections for double and single photoionization increase with hnu and reach saturated values of 0.78 at 85 eV for C(60) and approximately 1.3 at 100 eV for C(70). In contrast, the ratios at 120 eV between the cross sections for triple and single photoionization of C(60) and C(70) amount to 0.14 and approximately 0.38, respectively. The formation mechanism of multiply charged fullerene ions was discussed in terms of valence-electron excitation to antibonding unoccupied orbitals and/or spherical standing waves inside the cavity of a fullerene. This excitation could be followed by Spectator Auger processes and transmission of the excess electronic energy among numerous vibrational degrees of freedom.

  1. Photoionization Cross Section of Xe{sup +} Ion in the Pure 5p{sup 5} {sup 2}P{sub 3/2} Ground Level

    SciTech Connect

    Thissen, R.; Bizau, J. M.; Blancard, C.; Coreno, M.; Franceschi, P.; Giuliani, A.; Nicolas, C.

    2008-06-06

    Coupling an ion trap with synchrotron radiation is shown here to be a powerful approach to measure photoionization cross sections on ionic species relaxed in their ground state. The photoionization efficiency curve of Xe{sup +} ions stored in a Fourier transform ion cyclotron resonance ion trap was recorded at ELETTRA in the 20-23 eV photon energy range. Absolute cross sections were derived by comparison of the photoionization yield of Xe{sup +} with measurements from the ASTRID merged-beam experiment. Multiconfiguration Dirac-Fock calculations were performed for the interpretation of these new data.

  2. Differential cross-sections for the double photoionization of lithium

    NASA Astrophysics Data System (ADS)

    Kheifets, A. S.; Fursa, D. V.; Bray, Igor; Colgan, J.; Pindzola, M. S.

    2012-11-01

    We apply the convergent close-coupling (CCC) and time-dependent close- coupling (TDCC) methods to describe energy and angular resolved double photoionization (DPI) of lithium at arbitrary energy sharing. By doing so, we are able to evaluate the recoil ion momentum distribution of DPI of Li and make a comparison with recent measurements of Zhu et al. [Phys. Rev. Lett. 103, 103008 (2009)].

  3. Differential cross sections of double photoionization of lithium

    SciTech Connect

    Kheifets, A. S.; Fursa, D. V.; Bray, I.; Colgan, J.; Pindzola, M. S.

    2010-08-15

    We extend our previous application of the convergent close-coupling (CCC) and time-dependent close-coupling (TDCC) methods [Phys. Rev. A 81, 023418 (2010)] to describe energy and angular resolved double photoionization (DPI) of lithium at arbitrary energy sharing. By doing so, we are able to evaluate the recoil ion momentum distribution of DPI of Li and make a comparison with recent measurements of Zhu et al. [Phys. Rev. Lett. 103, 103008 (2009)].

  4. Calculation of photoionization cross section near auto-ionizing lines and magnesium photoionization cross section near threshold

    NASA Technical Reports Server (NTRS)

    Moore, E. N.; Altick, P. L.

    1972-01-01

    The research performed is briefly reviewed. A simple method was developed for the calculation of continuum states of atoms when autoionization is present. The method was employed to give the first theoretical cross section for beryllium and magnesium; the results indicate that the values used previously at threshold were sometimes seriously in error. These threshold values have potential applications in astrophysical abundance estimates.

  5. Differential cross sections of double photoionization of lithium

    NASA Astrophysics Data System (ADS)

    Kheifets, A. S.; Fursa, D. V.; Bray, I.; Colgan, J.; Pindzola, M. S.

    2010-08-01

    We extend our previous application of the convergent close-coupling (CCC) and time-dependent close-coupling (TDCC) methods [Phys. Rev. A10.1103/PhysRevA.81.023418 81, 023418 (2010)] to describe energy and angular resolved double photoionization (DPI) of lithium at arbitrary energy sharing. By doing so, we are able to evaluate the recoil ion momentum distribution of DPI of Li and make a comparison with recent measurements of Zhu [Phys. Rev. Lett.PRLTAO0031-900710.1103/PhysRevLett.103.103008 103, 103008 (2009)].

  6. Absolute vacuum ultraviolet photoabsorption cross section studies of atomic and molecular species: Techniques and observational data

    NASA Technical Reports Server (NTRS)

    Judge, D. L.; Wu, C. Y. R.

    1990-01-01

    Absorption of a high energy photon (greater than 6 eV) by an isolated molecule results in the formation of highly excited quasi-discrete or continuum states which evolve through a wide range of direct and indirect photochemical processes. These are: photoionization and autoionization, photodissociation and predissociation, and fluorescence. The ultimate goal is to understand the dynamics of the excitation and decay processes and to quantitatively measure the absolute partial cross sections for all processes which occur in photoabsorption. Typical experimental techniques and the status of observational results of particular interest to solar system observations are presented.

  7. Experimental verification of the individual energy dependencies of the partial L-shell photoionization cross sections of Pd and Mo.

    PubMed

    Hönicke, Philipp; Kolbe, Michael; Müller, Matthias; Mantler, Michael; Krämer, Markus; Beckhoff, Burkhard

    2014-10-17

    An experimental method for the verification of the individually different energy dependencies of L(1)-, L(2)-, and L(3)- subshell photoionization cross sections is described. The results obtained for Pd and Mo are well in line with theory regarding both energy dependency and absolute values, and confirm the theoretically calculated cross sections by Scofield from the early 1970 s and, partially, more recent data by Trzhaskovskaya, Nefedov, and Yarzhemsky. The data also demonstrate the questionability of quantitative x-ray spectroscopical results based on the widely used fixed jump ratio approximated cross sections with energy independent ratios. The experiments are carried out by employing the radiometrically calibrated instrumentation of the Physikalisch-Technische Bundesanstalt at the electron storage ring BESSY II in Berlin; the obtained fluorescent intensities are thereby calibrated at an absolute level in reference to the International System of Units. Experimentally determined fixed fluorescence line ratios for each subshell are used for a reliable deconvolution of overlapping fluorescence lines. The relevant fundamental parameters of Mo and Pd are also determined experimentally in order to calculate the subshell photoionization cross sections independently of any database.

  8. Hydrostatic pressure effect on photoionization cross section of a trion in quantum dots

    NASA Astrophysics Data System (ADS)

    Xie, Wenfang

    2013-11-01

    It is known experimentally that stable charged excitons can exist in low-dimensional semiconductor nanostructures. Much less is known about the properties of such charged-exciton complexes since three-body problems are very difficult to solve, even numerically. Here, we use the matrix diagonalization method and compact-density approach to investigate the charged excitons in a two-dimensional parabolic quantum dot. With typical semiconducting GaAs based materials, the photoionization cross section has been examined based on the computed energies and wave functions. We find that the photoionization cross section of charged excitons is strongly affected by the confinement frequency, hydrostatic pressure and temperature of QDs. Our results also show that the photoionization cross section of a negatively charged exciton is larger than that of a positively charged exciton.

  9. Dirac R-matrix calculations of photoionization cross-sections of Ni XIII

    NASA Astrophysics Data System (ADS)

    Sardar, S.; Bilal, M.; Bari, M. A.; Nazir, R. T.; Hannan, A.; Salahuddin, M.; Nasim, M. H.

    2016-05-01

    In this paper, we report total photoionization cross-sections of Ni XIII in the ground state (3P2) and four excited states (3P1,0, 1D2, 1S0) for the first time over the photon energy range 380-480 eV. The target wavefunctions are constructed with fully relativistic atomic structure GRASP code. Our calculated energy levels and oscillator strengths of core ion Ni XIV agree well with available experimental and theoretical results. The ionization threshold value of ground state of Ni XIII is found to be more closer to the experimental ionization energy and improved over the previous calculations. The photoionization cross-sections are calculated using the fully relativistic DARC code with an appropriate energy step of 0.01 eV to delineate the resonance structures. The calculated ionization cross-sections are important for the modelling of features of photoionized plasmas and for stellar opacities.

  10. Photoionization of Synchrotron-Radiation-Excited Atoms: Separating Partial Cross Sections by Full Polarization Control

    SciTech Connect

    Aloiese, S.; Meyer, M.; Cubaynes, D.; Grum-Grzhimailo, A. N.

    2005-06-10

    Resonant atomic excitation by synchrotron radiation and subsequent ionization by a tunable dye laser is used to study the photoionization of short-lived Rydberg states in Xe. By combining circular and linear polarization of the synchrotron as well as of the laser photons the partial photoionization cross sections were separated in the region of overlapping autoionizing resonances of different symmetry and the parameters of the resonances were extracted.

  11. Photoionization research on atomic radiation. 3: The ionization cross section of atomic nitrogen

    NASA Astrophysics Data System (ADS)

    Comes, F. J.; Elzer, A.

    1982-08-01

    The photoionization cross section of atomic nitrogen was measured between the ionization limit and 432 A. The experimental values are well fitted by those from a calculation of HENRY due to the dipole velocity approximation. A Rydberg series converging to the 5S-state of the ion is clearly identified from the ionization measurements and is shown to ionize.

  12. Measurement of photoionization cross sections of the excited states of titanium, cobalt, and nickel

    SciTech Connect

    Cong Ran; Cheng Yi; Yang Jiajun; Fan Jianmei; Yao Guanxin; Ji Xuehan; Zheng Xianfeng; Cui Zhifeng

    2009-07-01

    Resonance-enhanced multiphoton ionization (REMPI) of Ti, Co, and Ni atoms has been investigated in the 285-320 nm region. We couple a laser-ablated metal target into a molecular beam to produce atoms. Ions produced from photoionization of the neutral atoms are monitored by a home-built time-of-flight mass spectrometer. Photoionization cross sections of the excited states of Ti, Co, and Ni were deduced from the dependence of the ion signal intensity on the laser intensity for photon energies close to the ionization threshold. The values obtained range from 0.2 to 6.0 Mb. No significant isotope dependence was found from measurements of the photoionization cross sections of {sup 46}Ti, {sup 47}Ti, {sup 48}Ti, {sup 58}Ni, and {sup 60}Ni.

  13. Hartree-Fock calculation of the differential photoionization cross sections of small Li clusters

    SciTech Connect

    Galitskiy, S. A.; Artemyev, A. N.; Jänkälä, K.; Lagutin, B. M.; Demekhin, Ph. V.

    2015-01-21

    Cross sections and angular distribution parameters for the single-photon ionization of all electron orbitals of Li{sub 2−8} are systematically computed in a broad interval of the photoelectron kinetic energies for the energetically most stable geometry of each cluster. Calculations of the partial photoelectron continuum waves in clusters are carried out by the single center method within the Hartree-Fock approximation. We study photoionization cross sections per one electron and analyze in some details general trends in the photoionization of inner and outer shells with respect to the size and geometry of a cluster. The present differential cross sections computed for Li{sub 2} are in a good agreement with the available theoretical data, whereas those computed for Li{sub 3−8} clusters can be considered as theoretical predictions.

  14. Hartree-Fock calculation of the differential photoionization cross sections of small Li clusters.

    PubMed

    Galitskiy, S A; Artemyev, A N; Jänkälä, K; Lagutin, B M; Demekhin, Ph V

    2015-01-21

    Cross sections and angular distribution parameters for the single-photon ionization of all electron orbitals of Li2-8 are systematically computed in a broad interval of the photoelectron kinetic energies for the energetically most stable geometry of each cluster. Calculations of the partial photoelectron continuum waves in clusters are carried out by the single center method within the Hartree-Fock approximation. We study photoionization cross sections per one electron and analyze in some details general trends in the photoionization of inner and outer shells with respect to the size and geometry of a cluster. The present differential cross sections computed for Li2 are in a good agreement with the available theoretical data, whereas those computed for Li3-8 clusters can be considered as theoretical predictions.

  15. Absolute np and pp cross section determinations aimed at improving the standard for cross section measurements

    SciTech Connect

    Laptev, Alexander B; Haight, Robert C; Tovesson, Fredrik; Arndt, Richard A; Briscoe, William J; Paris, Mark W; Strakovsky, Igor I; Workman, Ron L

    2010-01-01

    Purpose of present research is a keeping improvement of the standard for cross section measurements of neutron-induced reactions. The cross sections for np and pp scattering below 1000 MeV are determined based on partial-wave analyses (PW As) of nucleon-nucleon scattering data. These cross sections are compared with the most recent ENDF/B-V11.0 and JENDL-4.0 data files, and the Nijmegen PWA. Also a comparison of evaluated data with recent experimental data was made to check a quality of evaluation. Excellent agreement was found between the new experimental data and our PWA predictions.

  16. Absolute np and pp Cross Section Determinations Aimed At Improving The Standard For Cross Section Measurements

    SciTech Connect

    Laptev, A. B.; Haight, R. C.; Tovesson, F.; Arndt, R. A.; Briscoe, W. J.; Paris, M. W.; Strakovsky, I. I.; Workman, R. L.

    2011-06-01

    Purpose of present research is a keeping improvement of the standard for cross section measurements of neutron-induced reactions. The cross sections for np and pp scattering below 1 GeV are determined based on partial-wave analyses (PWAs) of nucleon-nucleon scattering data. These cross sections are compared with the most recent ENDF/B-VII.0 and JENDL-4.0 data files, and the Nijmegen PWA. Also a comparison of evaluated data with recent experimental data was made to check a quality of evaluation. Excellent agreement was found between the new experimental data and our PWA predictions.

  17. Excitation energies, photoionization cross sections, and asymmetry parameters of the methyl and silyl radicals

    SciTech Connect

    Velasco, A. M.; Lavín, C.; Dolgounitcheva, O.; Ortiz, J. V.

    2014-08-21

    Vertical excitation energies of the methyl and silyl radicals were inferred from ab initio electron propagator calculations on the electron affinities of CH{sub 3}{sup +} and SiH{sub 3}{sup +}. Photoionization cross sections and angular distribution of photoelectrons for the outermost orbitals of both CH{sub 3} and SiH{sub 3} radicals have been obtained with the Molecular Quantum Defect Orbital method. The individual ionization cross sections corresponding to the Rydberg channels to which the excitation of the ground state's outermost electron gives rise are reported. Despite the relevance of methyl radical in atmospheric chemistry and combustion processes, only data for the photon energy range of 10–11 eV seem to be available. Good agreement has been found with experiment for photoionization cross section of this radical. To our knowledge, predictions of the above mentioned photoionization parameters on silyl radical are made here for the first time, and we are not aware of any reported experimental measurements. An analysis of our results reveals the presence of a Cooper minimum in the photoionization of the silyl radical. The adequacy of the two theoretical procedures employed in the present work is discussed.

  18. Dirac R-matrix calculations of photoionization cross-sections of Ca IV

    NASA Astrophysics Data System (ADS)

    Nazir, R. T.; Bari, M. A.; Sardar, S.; Bilal, M.; Salahuddin, M.; Nasim, M. H.

    2016-11-01

    In this paper total photoionization cross-sections in the ground (^2P^o_{3/2}) and two meta-stable states (^2P^o_{1/2},^2S_{1/2}) of Ca IV are reported using the relativistic Dirac Atomic R-matrix Codes (DARC) in the photon energy range 67-122 eV. The target wavefunctions are constructed with fully relativistic atomic structure GRASP package. A total of lowest lying 48 fine-structure levels arising from the four main configuration (3s23p4, 3s3p5 3s23p33d, 3p6) are considered for the target wavefunctions expansion. Our calculated eigenvalues of the core ion Ca V show reasonable agreement with available experimental and theoretical results. It is found that present ionization threshold energies of first three levels of Ca IV are in excellent agreement with NIST energies and experimental measurements. The photoionization cross-sections of Ca IV are calculated with an appropriate energy step (0.1 × 10-3 eV) to describe the resonance structures in vivid details. A comparison for the statistically weighted mixture of states (^2P^o_{3/2},^2P^o_{1/2}) with other experimental measurements including term-resolved ground state theoretical calculations is presented. Our computed photoionization cross-sections agree better with the measured cross-sections than the other theoretical approaches and are potentially more accurate.

  19. Parametrizations and dynamical analysis of angle-integrated cross sections for double photoionization including nondipole effects

    SciTech Connect

    Istomin, Andrei Y.; Starace, Anthony F.; Manakov, N. L.; Meremianin, A. V.; Kheifets, A. S.; Bray, Igor

    2005-11-15

    Similarly to differential cross sections for one-electron photoionization, the doubly differential cross section for double photoionization (DPI) may be conveniently described by four parameters: the singly differential (with respect to energy sharing) cross section ({sigma}{sub 0}), the dipole asymmetry parameter ({beta}), and two nondipole asymmetry parameters ({gamma} and {delta}). Here we derive two model-independent representations for these parameters for DPI from a {sup 1}S{sub 0} atomic bound state: (i) in terms of one-dimensional integrals of the polarization-invariant DPI amplitudes and (ii) in terms of the exact two-electron reduced matrix elements. For DPI of He at excess energies, E{sub exc}, of 100 eV, 450 eV, and 1 keV, we present numerical results for the asymmetry parameters within the framework of the convergent close-coupling theory and compare them with results of lowest-order (in the interelectron interaction) perturbation theory (LOPT). The results for E{sub exc}=1 keV exhibit a nondipole asymmetry that is large enough to be easily measured experimentally. We find excellent agreement between our LOPT results and other theoretical predictions and experimental data for total cross sections and ratios of double to single ionization cross sections for K-shell DPI from several multielectron atoms.

  20. Vibrationally specific photoionization cross sections of acrolein leading to the X̃²A' ionic state.

    PubMed

    López-Domínguez, Jesús A; Lucchese, Robert R; Fulfer, K D; Hardy, David; Poliakoff, E D; Aguilar, A A

    2014-09-07

    The vibrational branching ratios in the photoionization of acrolein for ionization leading to the X̃²A' ion state were studied. Computed logarithmic derivatives of the cross section and the corresponding experimental data derived from measured vibrational branching ratios for several normal modes (ν9, ν10, ν11, and ν12) were found to be in relatively good agreement, particularly for the lower half of the 11-100 eV photon energy range considered. Two shape resonances have been found near photon energies of 15.5 and 23 eV in the photoionization cross section and have been demonstrated to originate from the partial cross section of the A' scattering symmetry. The wave functions computed at the resonance complex energies are delocalized over the whole molecule. By looking at the dependence of the cross section on the different normal mode displacements together with the wave function at the resonant energy, a qualitative explanation is given for the change of the cross sections with respect to changing geometry.

  1. Photoionization cross-section of isotropic defects or impurity centers in isolators

    NASA Astrophysics Data System (ADS)

    Lima, H.; Batista, J. V.; Couto dos Santos, M. A.

    2016-08-01

    An analytical expression to calculate the photoionization cross-section of isotropic defects or impurity centers is being proposed by using the time-dependent perturbation theory. The ground-state wave function of the electron captured in the impurity state is described by a three-dimensional isotropic harmonic oscillator and the electron excited state in the continuum conduction band is described by a plane wave. The expression has been obtained considering all multipoles terms in the Hamiltonian, and that the radiation field which interacts with electrons is semi-classical and linearly polarized. This approximation is assumed because the effects of the linear contribution are dominant. The available data of the Al2O3:C and Lu2SiO5:Ce systems are in good agreement with our predictions. Such satisfactory comparison is a strong indication that the present model can be used to provide good predictions of the photoionization cross-section in several areas.

  2. Photoionization cross sections for atomic chlorine using an open-shell random phase approximation

    NASA Technical Reports Server (NTRS)

    Starace, A. F.; Armstrong, L., Jr.

    1975-01-01

    The use of the Random Phase Approximation with Exchange (RPAE) for calculating partial and total photoionization cross sections and photoelectron angular distributions for open shell atoms is examined for atomic chlorine. Whereas the RPAE corrections in argon (Z=18) are large, it is found that those in chlorine (Z=17) are much smaller due to geometric factors. Hartree-Fock calculations with and without core relaxation are also presented. Sizable deviations from the close coupling results of Conneely are also found.

  3. Parabolic versus spherical partial cross sections for photoionization excitation of He near threshold

    SciTech Connect

    Bouri, C.; Selles, P.; Malegat, L.; Kwato Njock, M. G.

    2006-09-15

    Spherical and parabolic partial cross sections and asymmetry parameters, defined in the ejected electron frame, are presented for photoionization excitation of the helium atom at 0.1 eV above its double ionization threshold. A quantitative law giving the dominant spherical partial wave l{sub dom} for each excitation level n is obtained. The parabolic partial cross sections are shown to satisfy the same approximate selection rules as the related Rydberg series of doubly excited states (K,T){sub n}{sup A}. The analysis of radial and angular correlations reveals the close relationship between double excitation, ionization excitation, and double ionization. Opposite to a widespread belief, the observed value of the asymmetry parameter is shown to result from the interplay of radial correlations and symmetry constraints, irrespective of angular correlations. Finally, the measurement of parabolic partial cross sections is proposed as a challenge to experimentalists.

  4. Vibrationally Resolved B 1s Photoionization Cross Section of BF3.

    PubMed

    Ayuso, D; Kimura, M; Kooser, K; Patanen, M; Plésiat, E; Argenti, L; Mondal, S; Travnikova, O; Sakai, K; Palacios, A; Kukk, E; Decleva, P; Ueda, K; Martín, F; Miron, C

    2015-06-11

    Photoelectron diffraction is a well-established technique for structural characterization of solids, based on the interference of the native photoelectron wave with those scattered from the neighboring atoms. For isolated systems in the gas phase similar studies suffer from orders of magnitude lower signals due to the very small sample density. Here we present a detailed study of the vibrationally resolved B 1s photoionization cross section of BF3 molecule. A combination of high-resolution photoelectron spectroscopy measurements and of state-of-the-art static-exchange and time-dependent DFT calculations shows the evolution of the photon energy dependence of the cross section from a complete trapping of the photoelectron wave (low energies) to oscillations due to photoelectron diffraction phenomena. The diffraction pattern allows one to access structural information both for the ground neutral state of the molecule and for the core-ionized cation. Due to a significant change in geometry between the ground and the B 1s(-1) core-ionized state in the BF3 molecule, several vibrational final states of the cation are populated, allowing investigation of eight different relative vibrationally resolved photoionization cross sections. Effects due to recoil induced by the photoelectron emission are also discussed.

  5. Band strength in photoelectron spectra and photoionization cross sections of pyrrole and of conformation isomers of 1,1-dimethylhydrazine

    SciTech Connect

    Kiro, Z. A.; Dykhanov, S. M.; Zverev, V. V.

    1988-09-01

    The dependence of partial photoionization cross sections of the 1,1-dimethylhydrazine molecule on the spatial characteristics (bond lengths, valence and dihedral angles) has been studied. The presence of a gauche-conformation isomer in the gaseous phase has been established, as confirmed by a comparison of the photoionization cross section ratios for the corresponding molecular orbitals with the relative band strengths in photoelectron spectra.

  6. Coherent correlation enhancement of outer shell photoionization cross sections of alkali-like ions

    SciTech Connect

    Amusia, M.Y.; Avdonina, B.; Pratt, R.H.

    1995-08-01

    An alkali-like ion interaction with inner electrons of an alkali-like ion leads to a significant increase in the photoionization cross section of the outer s electron. This occurs not only for ground-state ions with one s electron in the outer shell, but also when the outer s electron is in an excited state. The reason for this amplification, in addition to coherent enhancement in summing of the correlation amplitudes, is that the zero in the direct amplitude occurs below threshold. This leads to a constructive interference with the correlation amplitude above the photoionization threshold, in contrast to a destructive interference in the case of a neutral atom with the same electronic configuration, for which the zero occurs above threshold. Results of this research were published.

  7. Total molecular photoionization cross-sections by algebraic diagrammatic construction-Stieltjes-Lanczos method: Benchmark calculations

    NASA Astrophysics Data System (ADS)

    Ruberti, M.; Yun, R.; Gokhberg, K.; Kopelke, S.; Cederbaum, L. S.; Tarantelli, F.; Averbukh, V.

    2013-10-01

    In [K. Gokhberg, V. Vysotskiy, L. S. Cederbaum, L. Storchi, F. Tarantelli, and V. Averbukh, J. Chem. Phys. 130, 064104 (2009)] we introduced a new {L}2ab initio method for the calculation of total molecular photoionization cross-sections. The method is based on the ab initio description of discretized photoionized molecular states within the many-electron Green's function approach, known as algebraic diagrammatic construction (ADC), and on the application of Stieltjes-Chebyshev moment theory to Lanczos pseudospectra of the ADC electronic Hamiltonian. Here we establish the accuracy of the new technique by comparing the ADC-Lanczos-Stieltjes cross-sections in the valence ionization region to the experimental ones for a series of eight molecules of first row elements: HF, NH3, H2O, CO2, H2CO, CH4, C2H2, and C2H4. We find that the use of the second-order ADC technique [ADC(2)] that includes double electronic excitations leads to a substantial systematic improvement over the first-order method [ADC(1)] and to a good agreement with experiment for photon energies below 80 eV. The use of extended second-order ADC theory [ADC(2)x] leads to a smaller further improvement. Above 80 eV photon energy all three methods lead to significant deviations from the experimental values which we attribute to the use of Gaussian single-electron bases. Our calculations show that the ADC(2)-Lanczos-Stieltjes technique is a reliable and efficient ab initio tool for theoretical prediction of total molecular photo-ionization cross-sections in the valence region.

  8. Total molecular photoionization cross-sections by algebraic diagrammatic construction-Stieltjes-Lanczos method: benchmark calculations.

    PubMed

    Ruberti, M; Yun, R; Gokhberg, K; Kopelke, S; Cederbaum, L S; Tarantelli, F; Averbukh, V

    2013-10-14

    In [K. Gokhberg, V. Vysotskiy, L. S. Cederbaum, L. Storchi, F. Tarantelli, and V. Averbukh, J. Chem. Phys. 130, 064104 (2009)] we introduced a new L(2) ab initio method for the calculation of total molecular photoionization cross-sections. The method is based on the ab initio description of discretized photoionized molecular states within the many-electron Green's function approach, known as algebraic diagrammatic construction (ADC), and on the application of Stieltjes-Chebyshev moment theory to Lanczos pseudospectra of the ADC electronic Hamiltonian. Here we establish the accuracy of the new technique by comparing the ADC-Lanczos-Stieltjes cross-sections in the valence ionization region to the experimental ones for a series of eight molecules of first row elements: HF, NH3, H2O, CO2, H2CO, CH4, C2H2, and C2H4. We find that the use of the second-order ADC technique [ADC(2)] that includes double electronic excitations leads to a substantial systematic improvement over the first-order method [ADC(1)] and to a good agreement with experiment for photon energies below 80 eV. The use of extended second-order ADC theory [ADC(2)x] leads to a smaller further improvement. Above 80 eV photon energy all three methods lead to significant deviations from the experimental values which we attribute to the use of Gaussian single-electron bases. Our calculations show that the ADC(2)-Lanczos-Stieltjes technique is a reliable and efficient ab initio tool for theoretical prediction of total molecular photo-ionization cross-sections in the valence region.

  9. Photoionization cross section by Stieltjes imaging applied to coupled cluster Lanczos pseudo-spectra.

    PubMed

    Cukras, Janusz; Coriani, Sonia; Decleva, Piero; Christiansen, Ove; Norman, Patrick

    2013-09-07

    A recently implemented asymmetric Lanczos algorithm for computing (complex) linear response functions within the coupled cluster singles (CCS), coupled cluster singles and iterative approximate doubles (CC2), and coupled cluster singles and doubles (CCSD) is coupled to a Stieltjes imaging technique in order to describe the photoionization cross section of atoms and molecules, in the spirit of a similar procedure recently proposed by Averbukh and co-workers within the Algebraic Diagrammatic Construction approach. Pilot results are reported for the atoms He, Ne, and Ar and for the molecules H2, H2O, NH3, HF, CO, and CO2.

  10. Application of sampling theory in modelling of continuum processes: photoionization cross-sections of atoms

    NASA Astrophysics Data System (ADS)

    Kozlov, A.; Saha, S.; Quiney, H. M.

    2017-01-01

    We describe a method for the calculation of photoionization cross-sections using square-integrable amplitudes obtained from the diagonalization of finite-basis set representations of the electronic Hamiltonian. Three examples are considered: a model example in which the final state is a free particle, the hydrogen atom and neutral atomic sodium. The method exploits the Whittaker-Shannon-Kotel’nikov sampling theorem, which is widely used in digital signal sampling and reconstruction. The approach reproduces known data with very good accuracy and converges to the exact solution with increase of the basis set size.

  11. Photoionization cross section by Stieltjes imaging applied to coupled cluster Lanczos pseudo-spectra

    SciTech Connect

    Cukras, Janusz; Coriani, Sonia; Decleva, Piero; Christiansen, Ove; Norman, Patrick

    2013-09-07

    A recently implemented asymmetric Lanczos algorithm for computing (complex) linear response functions within the coupled cluster singles (CCS), coupled cluster singles and iterative approximate doubles (CC2), and coupled cluster singles and doubles (CCSD) is coupled to a Stieltjes imaging technique in order to describe the photoionization cross section of atoms and molecules, in the spirit of a similar procedure recently proposed by Averbukh and co-workers within the Algebraic Diagrammatic Construction approach. Pilot results are reported for the atoms He, Ne, and Ar and for the molecules H{sub 2}, H{sub 2}O, NH{sub 3}, HF, CO, and CO{sub 2}.

  12. Resonant and Near-Threshold Photoionization Cross Sections of Fe{sup 14+}

    SciTech Connect

    Simon, M. C.; Crespo Lopez-Urrutia, J. R.; Beilmann, C.; Schwarz, M.; Epp, S. W.; Schmitt, B. L.; Baumann, T. M.; Bernitt, S.; Ginzel, R.; Keitel, C. H.; Klawitter, R.; Kubicek, K.; Maeckel, V.; Mokler, P. H.; Ullrich, J.; Harman, Z.; Behar, E.; Follath, R.; Reichardt, G.; Schwarzkopf, O.

    2010-10-29

    Photoionization (PI) of Fe{sup 14+} in the range from 450 to 1100 eV was measured at the BESSY II storage ring using an electron beam ion trap achieving high target-ion area densities of 10{sup 10} cm{sup -2}. Photoabsorption by this ion is observed in astrophysical spectra and plasmas, but until now cross sections and resonance energies could only be provided by calculations. We reach a resolving power E/{Delta}E of at least 6500, outstanding in the present energy range, which enables benchmarking and improving the most advanced theories for PI of ions in high charge states.

  13. An X-Ray Analysis Database of Photoionization Cross Sections Including Variable Ionization

    NASA Technical Reports Server (NTRS)

    Wang, Ping; Cohen, David H.; MacFarlane, Joseph J.; Cassinelli, Joseph P.

    1997-01-01

    Results of research efforts in the following areas are discussed: review of the major theoretical and experimental data of subshell photoionization cross sections and ionization edges of atomic ions to assess the accuracy of the data, and to compile the most reliable of these data in our own database; detailed atomic physics calculations to complement the database for all ions of 17 cosmically abundant elements; reconciling the data from various sources and our own calculations; and fitting cross sections with functional approximations and incorporating these functions into a compact computer code.Also, efforts included adapting an ionization equilibrium code, tabulating results, and incorporating them into the overall program and testing the code (both ionization equilibrium and opacity codes) with existing observational data. The background and scientific applications of this work are discussed. Atomic physics cross section models and calculations are described. Calculation results are compared with available experimental data and other theoretical data. The functional approximations used for fitting cross sections are outlined and applications of the database are discussed.

  14. Absolute electron-impact total ionization cross sections of chlorofluoromethanes.

    PubMed

    Martínez, Roberto; Sierra, Borja; Redondo, Carolina; Rayo, María N Sánchez; Castaño, Fernando

    2004-12-15

    An experimental study is reported on the electron-impact total ionization cross sections (TICSs) of CCl4, CCl3F, CCl2F2, and CClF3 molecules. The kinetic energy of the colliding electrons was in the 10-85 eV range. TICSs were obtained as the sum of the partial ionization cross sections of all fragment ions, measured and identified in a linear double focusing time-of-flight mass spectrometer. The resulting TICS profiles--as a function of the electron-impact energy--have been compared both with those computed by ab initio and (semi)empirical methods and with the available experimental data. The computational methods used include the binary-encounter-Bethe (BEB) modified to include atoms with principal quantum numbers n> or =3, the Deutsch and Märk (DM) formalism, and the modified additivity rule (MAR). It is concluded that both modified BEB and DM methods fit the experimental TICS for (CF4), CClF3, CCl2F2, CCl3F, and CCl4 to a high accuracy, in contrast with the poor accord of the MAR method. A discussion on the factors influencing the discrepancies of the fittings is presented. (c) 2004 American Institute of Physics

  15. Absolute electron-impact total ionization cross sections of chlorofluoromethanes

    NASA Astrophysics Data System (ADS)

    Martínez, Roberto; Sierra, Borja; Redondo, Carolina; Rayo, María N. Sánchez; Castaño, Fernando

    2004-12-01

    An experimental study is reported on the electron-impact total ionization cross sections (TICSs) of CCl4, CCl3F, CCl2F2, and CClF3 molecules. The kinetic energy of the colliding electrons was in the 10-85 eV range. TICSs were obtained as the sum of the partial ionization cross sections of all fragment ions, measured and identified in a linear double focusing time-of-flight mass spectrometer. The resulting TICS profiles—as a function of the electron-impact energy—have been compared both with those computed by ab initio and (semi)empirical methods and with the available experimental data. The computational methods used include the binary-encounter-Bethe (BEB) modified to include atoms with principal quantum numbers n⩾3, the Deutsch and Märk (DM) formalism, and the modified additivity rule (MAR). It is concluded that both modified BEB and DM methods fit the experimental TICS for (CF4), CClF3, CCl2F2, CCl3F, and CCl4 to a high accuracy, in contrast with the poor accord of the MAR method. A discussion on the factors influencing the discrepancies of the fittings is presented.

  16. Absolute cross-section measurements for ionization of He Rydberg atoms in collisions with K

    NASA Astrophysics Data System (ADS)

    Deng, F.; Renwick, S.; Martínez, H.; Morgan, T. J.

    1995-11-01

    Absolute cross sections for ionization of 1.5-10.0 keV/amu Rydberg helium atoms in principal quantum states 12<=n<=15 due to collisions with potassium have been measured. The data are compared with the free-electron cross section at equal velocity. Our results for the collisional ionization cross sections (σi) agree both in shape and absolute magnitude with the data available for the total electron-scattering cross sections (σe) and support recent theoretical models for ionization of Rydberg atoms with neutral perturbers.

  17. Absolute cross-section normalization of magnetic neutron scattering data.

    PubMed

    Xu, Guangyong; Xu, Zhijun; Tranquada, J M

    2013-08-01

    We discuss various methods to obtain the resolution volume for neutron scattering experiments, in order to perform absolute normalization on inelastic magnetic neutron scattering data. Examples from previous experiments are given. We also try to provide clear definitions of a number of physical quantities which are commonly used to describe neutron magnetic scattering results, including the dynamic spin correlation function and the imaginary part of the dynamic susceptibility. Formulas that can be used for general purposes are provided and the advantages of the different normalization processes are discussed.

  18. Absolute cross-section normalization of magnetic neutron scattering data

    NASA Astrophysics Data System (ADS)

    Xu, Guangyong; Xu, Zhijun; Tranquada, J. M.

    2013-08-01

    We discuss various methods to obtain the resolution volume for neutron scattering experiments, in order to perform absolute normalization on inelastic magnetic neutron scattering data. Examples from previous experiments are given. We also try to provide clear definitions of a number of physical quantities which are commonly used to describe neutron magnetic scattering results, including the dynamic spin correlation function and the imaginary part of the dynamic susceptibility. Formulas that can be used for general purposes are provided and the advantages of the different normalization processes are discussed.

  19. Absolute UV absorption cross sections of dimethyl substituted Criegee intermediate (CH3)2COO

    NASA Astrophysics Data System (ADS)

    Chang, Yuan-Pin; Chang, Chun-Hung; Takahashi, Kaito; Lin, Jim-Min, Jr.

    2016-06-01

    The absolute absorption cross sections of (CH3)2COO under a jet-cooled condition were measured via laser depletion to be (1.32 ± 0.10) × 10-17 cm2 molecule-1 at 308 nm and (9.6 ± 0.8) × 10-18 cm2 molecule-1 at 352 nm. The peak UV cross section is estimated to be (1.75 ± 0.14) × 10-17 cm2 molecule-1 at 330 nm, according to the UV spectrum of (CH3)2COO (Huang et al., 2015) scaled to the absolute cross section at 308 nm.

  20. Absolute cross sections for dissociative electron attachment to NH3 and CH4

    NASA Astrophysics Data System (ADS)

    Rawat, Prashant; Prabhudesai, Vaibhav S.; Rahman, M. A.; Ram, N. Bhargava; Krishnakumar, E.

    2008-11-01

    Dissociative electron attachment (DEA) cross sections for NH3 and CH4 are measured in a crossed beam apparatus with special care to eliminate discrimination due to kinetic energy and angular distribution of the fragment ions. The cross sections are put on absolute scale using the relative flow technique. The absolute cross sections for the formation of H- and NH2- from ammonia and H- and CH2- from methane are compared with available data from literature. It is seen that the present results are considerably different 6rom what has been reported before. We also compare the cross sections of the H- channel from these molecules along with that from H2O to those from organic molecules containing alkyl, amino and hydroxyl groups to examine the extent to which the recently observed functional group dependence in the DEA contributes.

  1. Absolute metastable atom-atom collision cross section measurements using a magneto-optical trap.

    PubMed

    Matherson, K J; Glover, R D; Laban, D E; Sang, R T

    2007-07-01

    We present a new technique to measure absolute total collision cross sections from metastable neon atoms. The technique is based on the observation of the decay rate of trapped atoms as they collide with room temperature atoms. We present the first measurement of this kind using trapped neon atoms in the (3)P(2) metastable state colliding with thermal ground state argon. The measured cross section has a value of 556+/-26 A(2).

  2. Absolute differential cross sections for electron capture and loss by kilo-electron-volt hydrogen atoms

    NASA Technical Reports Server (NTRS)

    Smith, G. J.; Johnson, L. K.; Gao, R. S.; Smith, K. A.; Stebbings, R. F.

    1991-01-01

    This paper reports measurements of absolute differential cross sections for electron capture and loss for fast hydrogen atoms incident on H2, N2, O2, Ar, and He. Cross sections have been determined in the 2.0- to 5.0-keV energy range over the laboratory angular range 0.02-2 deg, with an angular, resolution of 0.02 deg. The high angular resolution allows observation of the structure at small angles in some of the cross sections. Comparison of the present results with those of other authors generally shows very good agreement.

  3. A general algorithm for fitting efficiently triple differential cross sections of atomic double photoionization

    NASA Astrophysics Data System (ADS)

    Argenti, Luca; Colle, Renato

    2008-12-01

    We propose an effective procedure to fit triple differential cross sections of atomic double photoionization processes, which is based on a general expression of the transition amplitude between arbitrary states of the target atom and the parent ion, with the transition operator expressed at any order of its multipolar expansion. The major advantage of our expression, which in the dipole approximation is equivalent to those of Manakov (1996 J. Phys. B: At. Mol. Opt. Phys. 29 2711) and Malegat (1997 J. Phys. B: At. Mol. Opt. Phys. 30 251), is that it is expressed only in terms of elementary angular functions (Clebsch-Gordan coefficients, spherical harmonics and 6 - j factors). Therefore our expression can be easily implemented in a general code for any kinematic condition and any order of the multipolar expansion of the transition operator. Our fitting procedure takes into account also the finite instrumental resolution in measuring energies and angles. Test calculations on helium and argon show that this further capability is often essential to remove important discrepancies between simulated and measured angular distributions.

  4. Nondipole effects in the triply differential cross section for double photoionization of He

    SciTech Connect

    Istomin, Andrei Y.; Starace, Anthony F.; Manakov, N.L.; Meremianin, A.V.

    2005-05-15

    Lowest-order nondipole effects are studied systematically in double photoionization (DPI) of the He atom. Ab initio parametrizations of the quadrupole transition amplitude for DPI from the {sup 1}S{sub 0} state are presented in terms of the exact two-electron radial matrix elements. Analytic expressions for these matrix elements within lowest-order perturbation theory (LOPT) in the interelectron interaction are also given. The corresponding parametrizations for the dipole-quadrupole triply differential cross section (TDCS) are presented for the case of an elliptically polarized photon. A general analysis of retardation-induced asymmetries of the TDCS including the circular dichroism effect at equal energy sharing is presented. Numerical LOPT estimates of nondipole asymmetries in photoelectron angular distributions for the cases of linear and circular polarization and of the circular dichroism effect at equal energy sharing are presented. We find that experimental observation of nondipole effects at excess energies of the order of tens to hundreds of eV should be feasible in TDCS measurements. Our numerical results exhibit a nondipole forward-backward asymmetry in the TDCS for DPI of He at an excess energy of 450 eV that is in qualitative agreement with existing experimental data.

  5. Calculation of photoionization differential cross sections using complex Gauss-type orbitals.

    PubMed

    Matsuzaki, Rei; Yabushita, Satoshi

    2017-09-05

    Accurate theoretical calculation of photoelectron angular distributions for general molecules is becoming an important tool to image various chemical reactions in real time. We show in this article that not only photoionization total cross sections but also photoelectron angular distributions can be accurately calculated using complex Gauss-type orbital (cGTO) basis functions. Our method can be easily combined with existing quantum chemistry techniques including electron correlation effects, and applied to various molecules. The so-called two-potential formula is applied to represent the transition dipole moment from an initial bound state to a final continuum state in the molecular coordinate frame. The two required continuum functions, the zeroth-order final continuum state and the first-order wave function induced by the photon field, have been variationally obtained using the complex basis function method with a mixture of appropriate cGTOs and conventional real Gauss-type orbitals (GTOs) to represent the continuum orbitals as well as the remaining bound orbitals. The complex orbital exponents of the cGTOs are optimized by fitting to the outgoing Coulomb functions. The efficiency of the current method is demonstrated through the calculations of the asymmetry parameters and molecular-frame photoelectron angular distributions of H2+ and H2 . In the calculations of H2 , the static exchange and random phase approximations are employed, and the dependence of the results on the basis functions is discussed. © 2017 Wiley Periodicals, Inc. © 2017 Wiley Periodicals, Inc.

  6. The Absolute Differential Cross-Section for Charge Transfer Scattering of 1.5 KEV Protons with Atomic Oxygen

    NASA Astrophysics Data System (ADS)

    Sieglaff, Dean Ronald

    The absolute cross section, differential in laboratory scattering angle, for the process rm H^ {+} + Oto H + O^{+} using 1.5 keV-energy protons is reported. The total cross section value of (8.7 +/- 1.9) times 10^{-16} cm^2 derived from the integration of the differential cross section is compared with existing cross section data.

  7. Configuration-interaction relativistic-many-body-perturbation-theory calculations of photoionization cross sections from quasicontinuum oscillator strengths

    SciTech Connect

    Savukov, I. M.; Filin, D. V.

    2014-12-29

    Many applications are in need of accurate photoionization cross sections, especially in the case of complex atoms. Configuration-interaction relativistic-many-body-perturbation theory (CI-RMBPT) has been successful in predicting atomic energies, matrix elements between discrete states, and other properties, which is quite promising, but it has not been applied to photoionization problems owing to extra complications arising from continuum states. In this paper a method that will allow the conversion of discrete CI-(R)MPBT oscillator strengths (OS) to photoionization cross sections with minimal modifications of the codes is introduced and CI-RMBPT cross sections of Ne, Ar, Kr, and Xe are calculated. A consistent agreement with experiment is found. RMBPT corrections are particularly significant for Ar, Kr, and Xe and improve agreement with experimental results compared to the particle-hole CI method. As a result, the demonstrated conversion method can be applied to CI-RMBPT photoionization calculations for a large number of multivalence atoms and ions.

  8. Configuration-interaction relativistic-many-body-perturbation-theory calculations of photoionization cross sections from quasicontinuum oscillator strengths

    DOE PAGES

    Savukov, I. M.; Filin, D. V.

    2014-12-29

    Many applications are in need of accurate photoionization cross sections, especially in the case of complex atoms. Configuration-interaction relativistic-many-body-perturbation theory (CI-RMBPT) has been successful in predicting atomic energies, matrix elements between discrete states, and other properties, which is quite promising, but it has not been applied to photoionization problems owing to extra complications arising from continuum states. In this paper a method that will allow the conversion of discrete CI-(R)MPBT oscillator strengths (OS) to photoionization cross sections with minimal modifications of the codes is introduced and CI-RMBPT cross sections of Ne, Ar, Kr, and Xe are calculated. A consistent agreementmore » with experiment is found. RMBPT corrections are particularly significant for Ar, Kr, and Xe and improve agreement with experimental results compared to the particle-hole CI method. As a result, the demonstrated conversion method can be applied to CI-RMBPT photoionization calculations for a large number of multivalence atoms and ions.« less

  9. Single and Triple Differential Cross Sections for DoublePhotoionization of H-

    SciTech Connect

    Yip, Frank L.; Horner, Daniel A.; McCurdy, C. William; Rescigno,Thomas N.

    2007-02-15

    The hydride anion H- would not be bound in the absence ofelectron correlation. Electron correlation drives the doublephotoionization process and, thus should impact double photoionizationresults most strongly for H-. We present fully differential crosssections for the three-body breakup of H- by single photon absorption.The absolute triple-differential and single-differential cross sectionswere yielded by ab initio calculations making use of exterior complexscaling within a discrete variable representation partialwave basis.Results calculated at photon energies of 18eV and 30eV are compared withreported cross sections for helium calculated at 20eV above the doubleionization threshold. These comparisons show a clear signature of initialstate correlation that differentiate the He and H- cases.

  10. Vibrationally specific photoionization cross sections of acrolein leading to the tilde{X} {}^2 A^' } ionic state

    NASA Astrophysics Data System (ADS)

    López-Domínguez, Jesús A.; Lucchese, Robert R.; Fulfer, K. D.; Hardy, David; Poliakoff, E. D.; Aguilar, A. A.

    2014-09-01

    The vibrational branching ratios in the photoionization of acrolein for ionization leading to the tilde{X} {}^2 A^' } ion state were studied. Computed logarithmic derivatives of the cross section and the corresponding experimental data derived from measured vibrational branching ratios for several normal modes (ν9, ν10, ν11, and ν12) were found to be in relatively good agreement, particularly for the lower half of the 11-100 eV photon energy range considered. Two shape resonances have been found near photon energies of 15.5 and 23 eV in the photoionization cross section and have been demonstrated to originate from the partial cross section of the A' scattering symmetry. The wave functions computed at the resonance complex energies are delocalized over the whole molecule. By looking at the dependence of the cross section on the different normal mode displacements together with the wave function at the resonant energy, a qualitative explanation is given for the change of the cross sections with respect to changing geometry.

  11. Absolute total and partial dissociative cross sections of pyrimidine at electron and proton intermediate impact velocities

    SciTech Connect

    Wolff, Wania Luna, Hugo; Sigaud, Lucas; Montenegro, Eduardo C.; Tavares, Andre C.

    2014-02-14

    Absolute total non-dissociative and partial dissociative cross sections of pyrimidine were measured for electron impact energies ranging from 70 to 400 eV and for proton impact energies from 125 up to 2500 keV. MOs ionization induced by coulomb interaction were studied by measuring both ionization and partial dissociative cross sections through time of flight mass spectrometry and by obtaining the branching ratios for fragment formation via a model calculation based on the Born approximation. The partial yields and the absolute cross sections measured as a function of the energy combined with the model calculation proved to be a useful tool to determine the vacancy population of the valence MOs from which several sets of fragment ions are produced. It was also a key point to distinguish the dissociation regimes induced by both particles. A comparison with previous experimental results is also presented.

  12. Absolute cross sections for dissociative electron attachment to H2O and D2O

    NASA Astrophysics Data System (ADS)

    Rawat, Prashant; Prabhudesai, Vaibhav S.; Aravind, G.; Rahman, M. A.; Krishnakumar, E.

    2007-12-01

    The dissociative electron attachment (DEA) process to water (H2O) and heavy water (D2O) has been studied in the gas phase in a cross beam experiment for electron energies up to 20 eV. The apparatus used eliminates discrimination due to the kinetic energy and angular distribution of the ions. The cross sections are normalized to absolute values using the cross section for production of O- from O2 (Rapp and Briglia 1965 J. Chem. Phys. 43 1480). These are the first exhaustive measurements of absolute cross sections for both the H- and O- from H2O and D- and O- from D2O at all the three resonances. The results are compared with the scarce data available in the literature. Isotope effect is observed at the 12 eV resonance in the H- channel and at all the three resonances in the O- channel.

  13. CaH Rydberg series, oscillator strengths and photoionization cross sections from Molecular Quantum Defect and Dyson Orbital theories

    NASA Astrophysics Data System (ADS)

    Velasco, A. M.; Lavín, C.; Díaz-Tinoco, Manuel; Ortiz, J. V.

    2017-01-01

    In this work, electron-propagator methods are applied to the calculation of the ionization potential and vertical excitation energies for several Rydberg series of the CaH molecule. The present calculations cover more highly excited states than those previously reported. In particular, excitation energies for ns (n>5), np (n>5), nd (n>4) and nf Rydberg states are given. Oscillator strengths for electronic transitions involving Rydberg states of CaH, as well as photoionization cross sections for Rydberg channels, also have been determined by using the Molecular Quantum Defect Orbital approach. Good agreement has been found with the scarce comparative data that are available for oscillator strengths. To our knowledge, predictions of photoionization cross sections from the outermost orbital of CaH are made here for the first time. A Cooper minimum and mixed atomic orbital character in some of the Dyson orbitals are among the novel features of these present calculations.

  14. Measurements of absolute absorption cross sections of ozone in the 185- to 254-nm wavelength region and the temperature dependence

    NASA Technical Reports Server (NTRS)

    Yoshino, K.; Esmond, J. R.; Freeman, D. E.; Parkinson, W. H.

    1993-01-01

    Laboratory measurements of the relative absorption cross sections of ozone at temperatures 195, 228, and 295 K have been made throughout the 185 to 254 nm wavelength region. The absolute absorption cross sections at the same temperatures have been measured at several discrete wavelengths in the 185 to 250 nm region. The absolute cross sections of ozone have been used to put the relative cross sections on a firm absolute basis throughout the 185 to 255 nm region. These recalibrated cross sections are slightly lower than those of Molina and Molina (1986), but the differences are within a few percent and would not be significant in atmospheric applications.

  15. Measurements of absolute absorption cross sections of ozone in the 185- to 254-nm wavelength region and the temperature dependence

    NASA Technical Reports Server (NTRS)

    Yoshino, K.; Esmond, J. R.; Freeman, D. E.; Parkinson, W. H.

    1993-01-01

    Laboratory measurements of the relative absorption cross sections of ozone at temperatures 195, 228, and 295 K have been made throughout the 185 to 254 nm wavelength region. The absolute absorption cross sections at the same temperatures have been measured at several discrete wavelengths in the 185 to 250 nm region. The absolute cross sections of ozone have been used to put the relative cross sections on a firm absolute basis throughout the 185 to 255 nm region. These recalibrated cross sections are slightly lower than those of Molina and Molina (1986), but the differences are within a few percent and would not be significant in atmospheric applications.

  16. Absolute measurement of the 242Pu neutron-capture cross section

    NASA Astrophysics Data System (ADS)

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; Bucher, B.; Chyzh, A.; Bredeweg, T. A.; Baramsai, B.; Couture, A.; Jandel, M.; Mosby, S.; O'Donnell, J. M.; Ullmann, J. L.; Dance Collaboration

    2016-04-01

    The absolute neutron-capture cross section of 242Pu was measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. The first direct measurement of the 242Pu(n ,γ ) cross section was made over the incident neutron energy range from thermal to ≈6 keV, and the absolute scale of the (n ,γ ) cross section was set according to the known 239Pu(n ,f ) resonance at En ,R=7.83 eV. This was accomplished by adding a small quantity of 239Pu to the 242Pu sample. The relative scale of the cross section, with a range of four orders of magnitude, was determined for incident neutron energies from thermal to ≈40 keV. Our data, in general, are in agreement with previous measurements and those reported in ENDF/B-VII.1; the 242Pu(n ,γ ) cross section at the En ,R=2.68 eV resonance is within 2.4 % of the evaluated value. However, discrepancies exist at higher energies; our data are ≈30 % lower than the evaluated data at En≈1 keV and are approximately 2 σ away from the previous measurement at En≈20 keV.

  17. Absolute X-ray emission cross section measurements of Fe K transitions

    NASA Astrophysics Data System (ADS)

    Hell, Natalie; Brown, Gregory V.; Beiersdorfer, Peter; Boyce, Kevin R.; Grinberg, Victoria; Kelley, Richard L.; Kilbourne, Caroline; Leutenegger, Maurice A.; Porter, Frederick Scott; Wilms, Jörn

    2016-06-01

    We have measured the absolute X-ray emission cross sections of K-shell transitions in highly charged L- and K-shell Fe ions using the LLNL EBIT-I electron beam ion trap and the NASA GSFC EBIT Calorimeter Spectrometer (ECS). The cross sections are determined by using the ECS to simultaneously record the spectrum of the bound-bound K-shell transitions and the emission from radiative recombination from trapped Fe ions. The measured spectrum is then brought to an absolute scale by normalizing the measured flux in the radiative recombination features to their theoretical cross sections, which are well known. Once the spectrum is brought to an absolute scale, the cross sections of the K-shell transitions are determined. These measurements are made possible by the ECS, which consists of a 32 channel array, with 14 channels optimized for detecting high energy photons (hν > 10 keV) and 18 channels optimized for detecting low energy photons (hν < 10 keV). The ECS has a large collection area, relatively high energy resolution, and a large bandpass; all properties necessary for this measurement technique to be successful. These data will be used to benchmark cross sections in the atomic reference data bases underlying the plasma modeling codes used to analyze astrophysical spectra, especially those measured by the Soft X-ray Spectrometer calorimeter instrument recently launched on the Hitomi X-ray Observatory.This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, and supported by NASA grants to LLNL and NASA/GSFC and by ESA under contract No. 4000114313/15/NL/CB.

  18. Absolute measurement of the 242Pu neutron-capture cross section

    DOE PAGES

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; ...

    2016-04-21

    Here, the absolute neutron-capture cross section of 242Pu was measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. The first direct measurement of the 242Pu(n,γ) cross section was made over the incident neutron energy range from thermal to ≈ 6 keV, and the absolute scale of the (n,γ) cross section was set according to the known 239Pu(n,f) resonance at En,R = 7.83 eV. This was accomplished by adding a small quantity of 239Pu to the 242Pu sample. The relative scale of the crossmore » section, with a range of four orders of magnitude, was determined for incident neutron energies from thermal to ≈ 40 keV. Our data, in general, are in agreement with previous measurements and those reported in ENDF/B-VII.1; the 242Pu(n,γ) cross section at the En,R = 2.68 eV resonance is within 2.4% of the evaluated value. However, discrepancies exist at higher energies; our data are ≈30% lower than the evaluated data at En ≈ 1 keV and are approximately 2σ away from the previous measurement at En ≈ 20 keV.« less

  19. Absolute measurements of electron capture cross sections of C3+ from atomic and molecular hydrogen

    NASA Astrophysics Data System (ADS)

    Sant'Anna, M. M.; Melo, W. S.; Santos, A. C. F.; Shah, M. B.; Sigaud, G. M.; Montenegro, E. C.

    2000-02-01

    Absolute measurements of single- and double-electron-capture cross sections by C3+ projectiles on atomic and molecular hydrogen targets were performed for projectile energies between 1.0 and 3.5 MeV for the single- and 1.0 and 2.0 MeV for the double-capture processes. The icons/Journals/Common/sigma" ALT="sigma" ALIGN="TOP"/> H /icons/Journals/Common/sigma" ALT="sigma" ALIGN="TOP"/> H2 cross section ratios were measured using an absolutely calibrated tungsten-tube furnace for the production of atomic hydrogen. The single-capture data are compared with calculations based on the boundary-corrected first Born approximation, the eikonal approximation and a semiclassical model, presenting a good overall agreement. Calculations for the double capture using an analytical expression, obtained within the independent electron approximation and based on the same semiclassical model, give a reasonable qualitative description of the data.

  20. Absolute determination of cross sections for resonant Raman scattering on silicon

    NASA Astrophysics Data System (ADS)

    Müller, Matthias; Beckhoff, Burkhard; Ulm, Gerhard; Kanngießer, Birgit

    2006-07-01

    We studied the resonant Raman scattering of x rays in the vicinity of the K absorption edge of silicon. The investigation was carried out at the plane grating monochromator beamline for undulator radiation of the PTB laboratory at BESSY II in Berlin. Cross sections were determined absolutely for a wide energy range of incident photons with small relative uncertainties employing calibrated instrumentation avoiding any reference samples. The experimentally determined values differ clearly from the theoretical ones found in the literature.

  1. Photoionization cross sections, electron-impact inverse mean free paths, and stopping powers for each subshell of silvera)

    NASA Astrophysics Data System (ADS)

    Lin, D. L.; Strickland, D. J.

    1980-03-01

    Using the Herman-Skillman potentials and bound wave functions for each subshell of silver, we have computed the continuum wave functions, and subshell-by-subshell photoionization cross sections with photoelectron energies up to 10 keV. Applying a relationship between photoionization and electron impact ionization, we have obtained inverse mean free paths and stopping powers, again by subshell, for electrons penetrating through silver. The maximum electron energy considered is 100 keV. For the total photoionization cross section, comparison of our work with experiment shows excellent agreement for photon energies down to 100 eV, below which solid-state effects should be included. Theoretical total inverse mean free paths, being strongly dominated by contributions from 4d electrons, are in good agreement with data around 1 keV, but about a factor of 2 larger at energies below 100eV. Our stopping power is in good agreement with other theoretical work above 400 eV and approaches the relativistic Bethe formula above 10 keV. Range is also computed and is in good agreement with other theoretical work.

  2. Absolute measurement of the 242Pu neutron-capture cross section

    SciTech Connect

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; Bucher, B.; Chyzh, A.; Bredeweg, T. A.; Baramsai, B.; Couture, A.; Jandel, M.; Mosby, S.; O'Donnell, J. M.; Ullmann, J. L.

    2016-04-21

    Here, the absolute neutron-capture cross section of 242Pu was measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. The first direct measurement of the 242Pu(n,γ) cross section was made over the incident neutron energy range from thermal to ≈ 6 keV, and the absolute scale of the (n,γ) cross section was set according to the known 239Pu(n,f) resonance at En,R = 7.83 eV. This was accomplished by adding a small quantity of 239Pu to the 242Pu sample. The relative scale of the cross section, with a range of four orders of magnitude, was determined for incident neutron energies from thermal to ≈ 40 keV. Our data, in general, are in agreement with previous measurements and those reported in ENDF/B-VII.1; the 242Pu(n,γ) cross section at the En,R = 2.68 eV resonance is within 2.4% of the evaluated value. However, discrepancies exist at higher energies; our data are ≈30% lower than the evaluated data at En ≈ 1 keV and are approximately 2σ away from the previous measurement at En ≈ 20 keV.

  3. Absolute measurement of the 242Pu neutron-capture cross section

    SciTech Connect

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; Bucher, B.; Chyzh, A.; Bredeweg, T. A.; Baramsai, B.; Couture, A.; Jandel, M.; Mosby, S.; O'Donnell, J. M.; Ullmann, J. L.

    2016-04-21

    Here, the absolute neutron-capture cross section of 242Pu was measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. The first direct measurement of the 242Pu(n,γ) cross section was made over the incident neutron energy range from thermal to ≈ 6 keV, and the absolute scale of the (n,γ) cross section was set according to the known 239Pu(n,f) resonance at En,R = 7.83 eV. This was accomplished by adding a small quantity of 239Pu to the 242Pu sample. The relative scale of the cross section, with a range of four orders of magnitude, was determined for incident neutron energies from thermal to ≈ 40 keV. Our data, in general, are in agreement with previous measurements and those reported in ENDF/B-VII.1; the 242Pu(n,γ) cross section at the En,R = 2.68 eV resonance is within 2.4% of the evaluated value. However, discrepancies exist at higher energies; our data are ≈30% lower than the evaluated data at En ≈ 1 keV and are approximately 2σ away from the previous measurement at En ≈ 20 keV.

  4. Absolute Cross Sections for Electron-Impact Ionization of Li-like Ions

    NASA Astrophysics Data System (ADS)

    Bannister, M. E.; Smith, A. C. H.; Djurić, N.; Wallbank, B.; Woitke, O.; Dunn, G. H.

    1998-05-01

    Absolute cross sections for the ionization of lithium-like B^2+ and C^3+ ions by electron-impact have been measured using a crossed-beams technique.(M. E. Bannister, Phys. Rev. A 54), 1435 (1996). Recently, several new sophisticated calculations(P. J. Marchalant et al), J. Phys. B 30, L435 (1997).^,( M. S. Pindzola and N. R. Badnell (private communication).) have been performed for B^2+ in an attempt to understand the disagreement between theory and previous experimental results,(D. H. Crandall et al.), Phys. Rev. A 34, 1757 (1986). a discrepancy of about 20% near the cross section peak. The present measurements for B^2+ are in very good agreement with these recent calculations and with the measurements of Hofmann et al.(G. Hofmann, A. Müller, K. Tinschert, and E. Salzborn, Z. Phys. D 16), 113 (1990). over the range that they report direct ionization cross sections. Experimental cross sections for ionization of C^3+ are also compared to recent theoretical predictions.

  5. Photoionization cross sections for O-like S IX: a Breit-Pauli R-matrix calculation

    NASA Astrophysics Data System (ADS)

    Tyndall, N. B.; Ramsbottom, C. A.; Hibbert, A.; Ferland, G.

    2015-08-01

    In this paper we present photoionization cross sections for the lowest five states of O-like S IX (1s22s22p4 3P0,1,2, 1D2, 1S0). The relativistic Breit-Pauli R-matrix codes were utilized including all terms of the 2s22p3, 2s2p4, 2p5, 2s22p23s, 3p, 3d and 2s2p33s, 3p, 3d configurations in the expansion of the collision wavefunction for S X. It was also found that to achieve convergence of the low-lying energy separations of the target levels, an additional 21 configuration functions needed to be included in the configuration interaction expansion, incorporating two-electron excitations from the 2s and 2p shells to the 3s, 3p and 3d shells. The present work thus constitutes the most sophisticated photoionization evaluation for ground and metastable levels of the S IX ion. Direct comparisons have been made with the only available data found on the OPEN-ADAS database between level resolved contributions of the spectrum. This comparison for the background cross section exhibits excellent agreement at all photon energies for each partial photoionization cross section contribution investigated. Finally, the autoionizing bound states arising from numerous open channels have also been investigated and identified using the QB approach, a procedure for analyzing resonances in atomic and molecular collision theory which exploits the analytic properties of R-matrix theory. Major Rydberg resonance series are also presented and tabulated for the dominant linewidths considered.

  6. Total photoionization cross-sections of excited electronic states by the algebraic diagrammatic construction-Stieltjes-Lanczos method

    NASA Astrophysics Data System (ADS)

    Ruberti, M.; Yun, R.; Gokhberg, K.; Kopelke, S.; Cederbaum, L. S.; Tarantelli, F.; Averbukh, V.

    2014-05-01

    Here, we extend the L2 ab initio method for molecular photoionization cross-sections introduced in Gokhberg et al. [J. Chem. Phys. 130, 064104 (2009)] and benchmarked in Ruberti et al. [J. Chem. Phys. 139, 144107 (2013)] to the calculation of total photoionization cross-sections of molecules in electronically excited states. The method is based on the ab initio description of molecular electronic states within the many-electron Green's function approach, known as algebraic diagrammatic construction (ADC), and on the application of Stieltjes-Chebyshev moment theory to Lanczos pseudospectra of the ADC electronic Hamiltonian. The intermediate state representation of the dipole operator in the ADC basis is used to compute the transition moments between the excited states of the molecule. We compare the results obtained using different levels of the many-body theory, i.e., ADC(1), ADC(2), and ADC(2)x for the first two excited states of CO, N2, and H2O both at the ground state and the excited state equilibrium or saddle point geometries. We find that the single excitation ADC(1) method is not adequate even at the qualitative level and that the inclusion of double electronic excitations for description of excited state photoionization is essential. Moreover, we show that the use of the extended ADC(2)x method leads to a substantial systematic difference from the strictly second-order ADC(2). Our calculations demonstrate that a theoretical modelling of photoionization of excited states requires an intrinsically double excitation theory with respect to the ground state and cannot be achieved by the standard single excitation methods with the ground state as a reference.

  7. Total photoionization cross-sections of excited electronic states by the algebraic diagrammatic construction-Stieltjes-Lanczos method.

    PubMed

    Ruberti, M; Yun, R; Gokhberg, K; Kopelke, S; Cederbaum, L S; Tarantelli, F; Averbukh, V

    2014-05-14

    Here, we extend the L2 ab initio method for molecular photoionization cross-sections introduced in Gokhberg et al. [J. Chem. Phys. 130, 064104 (2009)] and benchmarked in Ruberti et al. [J. Chem. Phys. 139, 144107 (2013)] to the calculation of total photoionization cross-sections of molecules in electronically excited states. The method is based on the ab initio description of molecular electronic states within the many-electron Green's function approach, known as algebraic diagrammatic construction (ADC), and on the application of Stieltjes-Chebyshev moment theory to Lanczos pseudospectra of the ADC electronic Hamiltonian. The intermediate state representation of the dipole operator in the ADC basis is used to compute the transition moments between the excited states of the molecule. We compare the results obtained using different levels of the many-body theory, i.e., ADC(1), ADC(2), and ADC(2)x for the first two excited states of CO, N2, and H2O both at the ground state and the excited state equilibrium or saddle point geometries. We find that the single excitation ADC(1) method is not adequate even at the qualitative level and that the inclusion of double electronic excitations for description of excited state photoionization is essential. Moreover, we show that the use of the extended ADC(2)x method leads to a substantial systematic difference from the strictly second-order ADC(2). Our calculations demonstrate that a theoretical modelling of photoionization of excited states requires an intrinsically double excitation theory with respect to the ground state and cannot be achieved by the standard single excitation methods with the ground state as a reference.

  8. Cross-section and asymmetry-parameter calculations for the outer- and inner-valence photoionization of ethane

    SciTech Connect

    Toffoli, Daniele; Simpson, Mary J.; Lucchese, Robert R.

    2004-06-01

    We have computed cross sections and asymmetry parameters for the outer- and inner-valence photoionization of ethane using the Schwinger variational method with Pade corrections. The calculated total cross section is found to be in rather good agreement with the available electron-impact and photoabsorption measurements. One-electron resonant processes in the (1e{sub g}){sup -1} (3a{sub 1g}){sup -1}, and (2a{sub 1g}){sup -1} ionization channels were examined comparing resonant states predicted from the virtual orbitals of a minimum basis set self-consistent-field (MBS-SCF) calculations with scattering resonances found using a local model potential for the electron-molecule interaction. The analysis of the interaction potential in terms of adiabatic radial components provides a description of the mechanism of the resonant trapping.

  9. Dissociative Recombination and Excitation of CH+5: Absolute Cross Sections and Branching Fractions

    NASA Astrophysics Data System (ADS)

    Semaniak, J.; Larson, Å.; Le Padellec, A.; Strömholm, C.; Larsson, M.; Rosén, S.; Peverall, R.; Danared, H.; Djuric, N.; Dunn, G. H.; Datz, S.

    1998-05-01

    The heavy-ion storage ring CRYRING was used to measure the absolute dissociative recombination and dissociative excitation cross sections for collision energies below 50 eV. Deduced thermal rates coefficients are consistent with previous beams data but are lower by a factor of 3 than the rates measured by means of the flowing afterglow Langmuir probe technique. A resonant structure in dissociative recombination cross section was found at 9 eV. We have determined the branching fractions in DR of CH+5 below 0.2 eV. The branching is dominated by three-body CH3 + H + H and CH2 + H2 + H dissociation channels, which occur with branching ratios of ~0.7 and ~0.2, respectively; thus methane is a minor species among dissociation products. Both the measured absolute cross sections and branching in dissociative recombination of CH+5 can have important implications for the models of dense interstellar clouds and abundance of CH2, CH3 and CH4 in these media.

  10. Absolute differential cross sections for elastic scattering of electrons from pyrimidine

    SciTech Connect

    Maljkovic, J. B.; Milosavljevic, A. R.; Sevic, D.; Marinkovic, B. P.; Blanco, F.

    2009-05-15

    Differential cross sections (DCSs) for elastic scattering of electrons from pyrimidine (C{sub 4}H{sub 4}N{sub 2}) are presented for incident energies from 50 to 300 eV. The measurements were performed using a cross beam technique, for scattering angles from 20 deg. to 110 deg. The relative DCSs were measured as a function of both the angle and incident energy and the absolute DCSs were determined using the relative flow method. The calculations of electron interaction cross sections are based on a corrected form of the independent-atom method, known as the screen corrected additivity rule procedure and using an improved quasifree absorption model. Calculated results agree very well with the experiment.

  11. Photoionization using the xchem approach: Total and partial cross sections of Ne and resonance parameters above the 2 s22 p5 threshold

    NASA Astrophysics Data System (ADS)

    Marante, Carlos; Klinker, Markus; Kjellsson, Tor; Lindroth, Eva; González-Vázquez, Jesús; Argenti, Luca; Martín, Fernando

    2017-08-01

    The XCHEM approach interfaces well established quantum chemistry packages with scattering numerical methods in order to describe single-ionization processes in atoms and molecules. This should allow one to describe electron correlation in the continuum at the same level of accuracy as quantum chemistry methods do for bound states. Here we have applied this method to study multichannel photoionization of Ne in the vicinity of the autoionizing states lying between the 2 s22 p5 and 2 s 2 p6 ionization thresholds. The calculated total photoionization cross sections are in very good agreement with the absolute measurement of Samson et al. [J. Electron Spectrosc. Relat. Phenom. 123, 265 (2002), 10.1016/S0368-2048(02)00026-9], and with independent benchmark calculations performed at the same level of theory. From these cross sections, we have extracted resonance positions, total autoionization widths, Fano profile parameters, and correlation parameters for the lowest three autoionizing states. The values of these parameters are in good agreement with those reported in earlier theoretical and experimental work. We have also evaluated β asymmetry parameter and partial photoionization cross sections and, from the latter, partial autoionization widths and Starace parameters for the same resonances, not yet available in the literature. Resonant features in the calculated β parameter are in good agreement with the experimental observations. We have found that the three lowest resonances preferentially decay into the 2 p-1ɛ d continuum rather than into the 2 p-1ɛ s one [Phys. Rev. A 89, 043415 (2014), 10.1103/PhysRevA.89.043415], in agreement with previous expectations, and that in the vicinity of the resonances the partial 2 p-1ɛ s cross section can be larger than the 2 p-1ɛ d one, in contrast with the accepted idea that the latter should amply dominate in the whole energy range. These results show the potential of the XCHEM approach to describe highly correlated process

  12. Influence of shape resonances on minima in cross sections for photoionization of excited atoms

    SciTech Connect

    Felfli, Z.; Manson, S.T. Department of Astronomy, Georgia State University, Atlanta, Georgia 30303 )

    1990-02-01

    A relationship between the location of Cooper minima and the difference between the quantum defect of the initial state and the threshold phase shift (in units of {pi}) of the final state in excited photoionization has been suggested earlier (Phys. Rev. Lett. 48, 473 (1982)). The existence of a shape resonance in the final state is shown to modify this relationship.

  13. Dirac R-matrix calculations of photoionization cross sections of Ni XII and atomic structure data of Ni XIII

    NASA Astrophysics Data System (ADS)

    Nazir, R. T.; Bari, M. A.; Bilal, M.; Sardar, S.; Nasim, M. H.; Salahuddin, M.

    2017-02-01

    We performed R-matrix calculations for photoionization cross sections of the two ground state configuration 3s23p5 (^2P^o3/2,1/2) levels and 12 excited states of Ni XII using relativistic Dirac Atomic R-matrix Codes (DARC) across the photon energy range between the ionizations thresholds of the corresponding states and well above the thresholds of the last level of the Ni XIII target ion. Generally, a good agreement is obtained between our results and the earlier theoretical photoionization cross sections. Moreover, we have used two independent fully relativistic GRASP and FAC codes to calculate fine-structure energy levels, wavelengths, oscillator strengths, transitions rates among the lowest 48 levels belonging to the configuration (3s23p4, 3s3p5, 3p6, 3s23p33d) in Ni XIII. Additionally, radiative lifetimes of all the excited states of Ni XIII are presented. Our results of the atomic structure of Ni XIII show good agreement with other theoretical and experimental results available in the literature. A good agreement is found between our calculated lifetimes and the experimental ones. Our present results are useful for plasma diagnostic of fusion and astrophysical plasmas.

  14. Absolute differential cross sections for elastic electron scattering from small biomolecules

    NASA Astrophysics Data System (ADS)

    Maljković, Jelena

    2014-12-01

    The results of an experimental investigation of electrons colliding with a set of biomolecules that are assumed to be analogues of the building blocks of DNA (furan, 3- hydroxytetrahydrofuran and pyrimidine) and proteins (formamide, N-methylformamide) are presented. Absolute differential cross sections at medium incident electron energies 40 eV- 300 eV are presented and compared for these different targets. The experimental results are also compared with available calculations, based on the corrected form of independent atom model and show good agreement over the energy range studied.

  15. Relative Photoionization Cross Sections of Super-Atom Molecular Orbitals (SAMOs) in C60.

    PubMed

    Bohl, Elvira; Sokół, Katarzyna P; Mignolet, Benoit; Thompson, James O F; Johansson, J Olof; Remacle, Francoise; Campbell, Eleanor E B

    2015-11-25

    The electronic structure and photoinduced dynamics of fullerenes, especially C60, is of great interest because these molecules are model systems for more complex molecules and nanomaterials. In this work we have used Rydberg Fingerprint Spectroscopy to determine the relative ionization intensities from excited SAMO (Rydberg-like) states in C60 as a function of laser wavelength. The relative ionization intensities are then compared to the ratio of the photoionization widths of the Rydberg-like states, computed in time-dependent density functional theory (TD-DFT). The agreement is remarkably good when the same photon order is required to energetically access the excited states. This illustrates the predictive potential of quantum chemistry for studying photoionization of large, complex molecules as well as confirming the assumption that is often made concerning the multiphoton excitation and rapid energy redistribution in the fullerenes.

  16. Absolute photo-destruction and photo-fragmentation cross section measurements using an electrostatic ion beam trap.

    PubMed

    Aviv, O; Kafle, B; Chandrasekaran, V; Heber, O; Rappaport, M L; Rubinstein, H; Schwalm, D; Strasser, D; Toker, Y; Zajfman, D

    2013-05-01

    We describe a technique to measure absolute photo-induced cross sections for cluster anions stored in an electrostatic ion beam trap (EIBT) with a central deflector. The setup allows determination of total photo-destruction cross sections as well as partial cross sections for fragmentation and electron detachment. The unique properties of this special EIBT setup are investigated and illustrated using small Al(n)(-) clusters.

  17. Explanation of observed interference patterns in the differential cross section for double photoionization of H2

    SciTech Connect

    Horner, Daniel A; Miyabe, Shungo; Morales, Felipe; Martin, Fernando; Rescigno, Thomas N; Mccurdy, C William

    2009-01-01

    We present the results of numerical calculations on the single photon double photoionization of H{sub 2} for energies between 130 eV and 240 eV. We find that our results are in excellent agreement with experimental observations. However, our interpretation of the observed interference pattern at these energies is that it is due to mixing of parallel and perpendicular components through circularly polarized light rather than due to classical double slit diffraction.

  18. Systematic determination of absolute absorption cross-section of individual carbon nanotubes.

    PubMed

    Liu, Kaihui; Hong, Xiaoping; Choi, Sangkook; Jin, Chenhao; Capaz, Rodrigo B; Kim, Jihoon; Wang, Wenlong; Bai, Xuedong; Louie, Steven G; Wang, Enge; Wang, Feng

    2014-05-27

    Optical absorption is the most fundamental optical property characterizing light-matter interactions in materials and can be most readily compared with theoretical predictions. However, determination of optical absorption cross-section of individual nanostructures is experimentally challenging due to the small extinction signal using conventional transmission measurements. Recently, dramatic increase of optical contrast from individual carbon nanotubes has been successfully achieved with a polarization-based homodyne microscope, where the scattered light wave from the nanostructure interferes with the optimized reference signal (the reflected/transmitted light). Here we demonstrate high-sensitivity absorption spectroscopy for individual single-walled carbon nanotubes by combining the polarization-based homodyne technique with broadband supercontinuum excitation in transmission configuration. To our knowledge, this is the first time that high-throughput and quantitative determination of nanotube absorption cross-section over broad spectral range at the single-tube level was performed for more than 50 individual chirality-defined single-walled nanotubes. Our data reveal chirality-dependent behaviors of exciton resonances in carbon nanotubes, where the exciton oscillator strength exhibits a universal scaling law with the nanotube diameter and the transition order. The exciton linewidth (characterizing the exciton lifetime) varies strongly in different nanotubes, and on average it increases linearly with the transition energy. In addition, we establish an empirical formula by extrapolating our data to predict the absorption cross-section spectrum for any given nanotube. The quantitative information of absorption cross-section in a broad spectral range and all nanotube species not only provides new insight into the unique photophysics in one-dimensional carbon nanotubes, but also enables absolute determination of optical quantum efficiencies in important

  19. Systematic determination of absolute absorption cross-section of individual carbon nanotubes

    PubMed Central

    Liu, Kaihui; Hong, Xiaoping; Choi, Sangkook; Jin, Chenhao; Capaz, Rodrigo B.; Kim, Jihoon; Wang, Wenlong; Bai, Xuedong; Louie, Steven G.; Wang, Enge; Wang, Feng

    2014-01-01

    Optical absorption is the most fundamental optical property characterizing light–matter interactions in materials and can be most readily compared with theoretical predictions. However, determination of optical absorption cross-section of individual nanostructures is experimentally challenging due to the small extinction signal using conventional transmission measurements. Recently, dramatic increase of optical contrast from individual carbon nanotubes has been successfully achieved with a polarization-based homodyne microscope, where the scattered light wave from the nanostructure interferes with the optimized reference signal (the reflected/transmitted light). Here we demonstrate high-sensitivity absorption spectroscopy for individual single-walled carbon nanotubes by combining the polarization-based homodyne technique with broadband supercontinuum excitation in transmission configuration. To our knowledge, this is the first time that high-throughput and quantitative determination of nanotube absorption cross-section over broad spectral range at the single-tube level was performed for more than 50 individual chirality-defined single-walled nanotubes. Our data reveal chirality-dependent behaviors of exciton resonances in carbon nanotubes, where the exciton oscillator strength exhibits a universal scaling law with the nanotube diameter and the transition order. The exciton linewidth (characterizing the exciton lifetime) varies strongly in different nanotubes, and on average it increases linearly with the transition energy. In addition, we establish an empirical formula by extrapolating our data to predict the absorption cross-section spectrum for any given nanotube. The quantitative information of absorption cross-section in a broad spectral range and all nanotube species not only provides new insight into the unique photophysics in one-dimensional carbon nanotubes, but also enables absolute determination of optical quantum efficiencies in important

  20. Dissociative Recombination of D3S+: Product Branching Fractions and Absolute Cross Sections

    NASA Astrophysics Data System (ADS)

    Kamińska, M.; Vigren, E.; Zhaunerchyk, V.; Geppert, W. D.; Roberts, H.; Walsh, C.; Millar, T. J.; Danielsson, M.; Hamberg, M.; Thomas, R. D.; Larsson, M.; Ugglas, M. af; Semaniak, J.

    2008-07-01

    The dissociative recombination (DR) of D3S+ has been studied at the heavy ion storage ring CRYRING. The absolute DR cross sections have been measured over the interaction energy range between ~0 and 0.1 eV, and the energy-dependent cross section obtained is best fitted by the expression σ (E) = (1.3 +/- 0.3) × 10-16E-1.36 +/- 0.04 cm2. From the cross section the thermal rate coefficient has been deduced to be (2.8 +/- 0.7) × 10-7(T/300)-0.86 +/- 0.03 cm3 s-1. The branching fractions in the reaction have been measured at ~0 eV collision energy. The break-up into D2S+D occurs with a probability of only 0.17 +/- 0.08, whereas the three-body channel DS+2D dominates with a probability of 0.58 +/- 0.11. The remaining channels DS+D2 and S+D2+D contribute with 0.15 +/- 0.07 and 0.10 +/- 0.06, respectively. The impact of these results on the sulfur chemistry and deuterium fractionation in dark molecular clouds was investigated through chemical kinetic models. With these data, the calculated fractional abundance of H2S is lower than observed in TMC-1, which supports the assertion that H2S is formed on grain surfaces and not through gas-phase reactions.

  1. Optimization of complex slater-type functions with analytic derivative methods for describing photoionization differential cross sections.

    PubMed

    Matsuzaki, Rei; Yabushita, Satoshi

    2017-05-05

    The complex basis function (CBF) method applied to various atomic and molecular photoionization problems can be interpreted as an L2 method to solve the driven-type (inhomogeneous) Schrödinger equation, whose driven term being dipole operator times the initial state wave function. However, efficient basis functions for representing the solution have not fully been studied. Moreover, the relation between their solution and that of the ordinary Schrödinger equation has been unclear. For these reasons, most previous applications have been limited to total cross sections. To examine the applicability of the CBF method to differential cross sections and asymmetry parameters, we show that the complex valued solution to the driven-type Schrödinger equation can be variationally obtained by optimizing the complex trial functions for the frequency dependent polarizability. In the test calculations made for the hydrogen photoionization problem with five or six complex Slater-type orbitals (cSTOs), their complex valued expansion coefficients and the orbital exponents have been optimized with the analytic derivative method. Both the real and imaginary parts of the solution have been obtained accurately in a wide region covering typical molecular regions. Their phase shifts and asymmetry parameters are successfully obtained by extrapolating the CBF solution from the inner matching region to the asymptotic region using WKB method. The distribution of the optimized orbital exponents in the complex plane is explained based on the close connection between the CBF method and the driven-type equation method. The obtained information is essential to constructing the appropriate basis sets in future molecular applications. © 2017 Wiley Periodicals, Inc.

  2. Absolute angle-differential vibrational excitation cross sections for electron collisions with diacetylene

    SciTech Connect

    Allan, M.; May, O.; Fedor, J.; Ibanescu, B. C.; Andric, L.

    2011-05-15

    Absolute vibrational excitation cross sections were measured for diacetylene (1,3-butadiyne). The selectivity of vibrational excitation reveals detailed information about the shape resonances. Excitation of the C{identical_to}C stretch and of double quanta of the C-H bend vibrations reveals a {sup 2}{Pi}{sub u} resonance at 1 eV (autodetachment width {approx}30 meV) and a {sup 2}{Pi}{sub g} resonance at 6.2 eV (autodetachment width 1-2 eV). There is a strong preference for excitation of even quanta of the bending vibration. Excitation of the C-H stretch vibration reveals {sigma}* resonances at 4.3, 6.8, and 9.8 eV, with autodetachment widths of {approx}2 eV. Detailed information about resonances permits conclusions about the mechanism of the dissociative electron attachment.

  3. Absolute cross sections for ethylene-dication production by electron impact

    NASA Astrophysics Data System (ADS)

    Sigaud, L.; Montenegro, E. C.

    2017-01-01

    This work reports absolute cross-section measurements for the production of ethylene dications by electron impact, with the energy ranging between 25 and 800 eV. Separation of the entangled C2H42 + and CH2+ fragments with the same mass-to-charge ratio, in the time-of-flight spectrum, is properly carried out using the DETOF technique. This separation shows that stable C2H42 + can be produced either by two primary vacancies or by a single primary vacancy in an inner valence shell, with its subsequent de-excitation through Auger-like decay. Our findings show that the latter process can be an important player in dication formation, prevailing in the case of ethylene at projectile energies above 500 eV.

  4. B-spline algebraic diagrammatic construction: application to photoionization cross-sections and high-order harmonic generation.

    PubMed

    Ruberti, M; Averbukh, V; Decleva, P

    2014-10-28

    We present the first implementation of the ab initio many-body Green's function method, algebraic diagrammatic construction (ADC), in the B-spline single-electron basis. B-spline versions of the first order [ADC(1)] and second order [ADC(2)] schemes for the polarization propagator are developed and applied to the ab initio calculation of static (photoionization cross-sections) and dynamic (high-order harmonic generation spectra) quantities. We show that the cross-section features that pose a challenge for the Gaussian basis calculations, such as Cooper minima and high-energy tails, are found to be reproduced by the B-spline ADC in a very good agreement with the experiment. We also present the first dynamic B-spline ADC results, showing that the effect of the Cooper minimum on the high-order harmonic generation spectrum of Ar is correctly predicted by the time-dependent ADC calculation in the B-spline basis. The present development paves the way for the application of the B-spline ADC to both energy- and time-resolved theoretical studies of many-electron phenomena in atoms, molecules, and clusters.

  5. B-spline algebraic diagrammatic construction: Application to photoionization cross-sections and high-order harmonic generation

    SciTech Connect

    Ruberti, M.; Averbukh, V.; Decleva, P.

    2014-10-28

    We present the first implementation of the ab initio many-body Green's function method, algebraic diagrammatic construction (ADC), in the B-spline single-electron basis. B-spline versions of the first order [ADC(1)] and second order [ADC(2)] schemes for the polarization propagator are developed and applied to the ab initio calculation of static (photoionization cross-sections) and dynamic (high-order harmonic generation spectra) quantities. We show that the cross-section features that pose a challenge for the Gaussian basis calculations, such as Cooper minima and high-energy tails, are found to be reproduced by the B-spline ADC in a very good agreement with the experiment. We also present the first dynamic B-spline ADC results, showing that the effect of the Cooper minimum on the high-order harmonic generation spectrum of Ar is correctly predicted by the time-dependent ADC calculation in the B-spline basis. The present development paves the way for the application of the B-spline ADC to both energy- and time-resolved theoretical studies of many-electron phenomena in atoms, molecules, and clusters.

  6. Measurements of absolute total and partial cross sections for the electron ionization of tungsten hexafluoride (WF6)

    NASA Astrophysics Data System (ADS)

    Basner, R.; Schmidt, M.; Becker, K.

    2004-04-01

    We measured absolute partial cross sections for the formation of positive ions followed by electron impact on tungsten hexafluoride (WF6) from threshold to 900 eV using a time-of-flight mass spectrometer (TOF-MS). Dissociative ionization processes resulting in seven different singly charged ions (F+, W+, WFx+, x=1-5) and five doubly charged ions (W2+, WFx2+, x=1-4) were found to be the dominant ionization channels. The ion spectrum at all impact energies is dominated by WF5+ fragment ions. At 120 eV impact energy, the partial WF5+ ionization cross section has a maximum value of 3.92×10-16 cm2 that corresponds to 43% of the total ion yield. The cross section values of all the other singly charged fragment ions at 120 eV range between 0.39×10-16 and 0.73×10-16 cm2. The ionization cross sections of the doubly charged ions are more than one order of magnitude lower than the cross section of WF5+. Double ionization processes account for 21% of the total ion yield at 120 eV. The absolute total ionization cross section of WF6 was obtained as the sum of all measured partial ionization cross sections and is compared with available calculated cross sections.

  7. Absolute Differential Scattering Cross-Sections of Electrons from Neon, Nitrogen and Methyl Chloride

    NASA Astrophysics Data System (ADS)

    Shi, Xueying

    The relative flow technique is used to obtain absolute DCS in a crossed-beam experiment. A novel gas handling system was designed to facilitate these measurements. The absolute DCS of electrons scattered from neon have been measured from 7 eV down to 0.25 eV. At energies of 2 eV and lower, our results are in excellent agreement with MERT and recent ab initio calculation. At energies higher than 2 eV, our results are in excellent agreement with those of Williams. Thus we propose that neon can be used as a benchmark to test the overall performance of the electron spectrometer at low energies. The angular dependence of absolute vibrationally -elastic DCS of electrons scattered from N_2 have been measured at 0.55 eV, 1.50 eV, and ~2.22 eV, the second elastic peak of the ^2Pi_{rm g} resonance. Our results at these two lower energies are much larger than the previous experimental results, but in close agreement with theoretical calculations by Morrison. By extrapolating our curves to 0^ circ and 180^circ using Morrison's curves as a guide, integration gave the total vibrationally-elastic cross sections at these two energies. Our results are within 2-4% of the experimentally measured total cross sections. Methyl Chloride is the simplest saturated hydrocarbon with a single chlorine atom substitution. Two resonances have been assigned in CH_3Cl, the a_1(C-Cl,sigma^*) resonance at 3.45 eV and the e(C-H,sigma ^*) resonance at 5.5 eV. In the elastic channel, the measurements show that dipole scattering dominates at low energies and in the forward direction. In inelastic channels, the C-Cl stretch mode nu_3(a _1) is strongly excited by the sigma ^*(C-Cl) shape resonance, and the C-H stretch mode nu_4(e) is the strongest one excited by the e resonance. The angular dependences for excitation of these two modes are relatively flat. The shapes cannot be explained solely by a few leading terms in the angular momentum expansion arising from the resonance. This suggests that non

  8. Absolute cross-sections for DNA strand breaks and crosslinks induced by low energy electrons.

    PubMed

    Chen, Wenzhuang; Chen, Shiliang; Dong, Yanfang; Cloutier, Pierre; Zheng, Yi; Sanche, Léon

    2016-12-07

    Absolute cross sections (CSs) for the interaction of low energy electrons with condensed macromolecules are essential parameters to accurately model ionizing radiation induced reactions. To determine CSs for various conformational DNA damage induced by 2-20 eV electrons, we investigated the influence of the attenuation length (AL) and penetration factor (f) using a mathematical model. Solid films of supercoiled plasmid DNA with thicknesses of 10, 15 and 20 nm were irradiated with 4.6, 5.6, 9.6 and 14.6 eV electrons. DNA conformational changes were quantified by gel electrophoresis, and the respective yields were extrapolated from exposure-response curves. The absolute CS, AL and f values were generated by applying the model developed by Rezaee et al. The values of AL were found to lie between 11 and 16 nm with the maximum at 14.6 eV. The absolute CSs for the loss of the supercoiled (LS) configuration and production of crosslinks (CL), single strand breaks (SSB) and double strand breaks (DSB) induced by 4.6, 5.6, 9.6 and 14.6 eV electrons are obtained. The CSs for SSB are smaller, but similar to those for LS, indicating that SSB are the main conformational damage. The CSs for DSB and CL are about one order of magnitude smaller than those of LS and SSB. The value of f is found to be independent of electron energy, which allows extending the absolute CSs for these types of damage within the range 2-20 eV, from previous measurements of effective CSs. When comparison is possible, the absolute CSs are found to be in good agreement with those obtained from previous similar studies with double-stranded DNA. The high values of the absolute CSs of 4.6 and 9.6 eV provide quantitative evidence for the high efficiency of low energy electrons to induce DNA damage via the formation of transient anions.

  9. Absolute total and partial cross sections for ionization of nucleobases by proton impact in the Bragg peak velocity range

    SciTech Connect

    Tabet, J.; Eden, S.; Feil, S.; Abdoul-Carime, H.; Farizon, B.; Farizon, M.; Ouaskit, S.; Maerk, T. D.

    2010-08-15

    We present experimental results for proton ionization of nucleobases (adenine, cytosine, thymine, and uracil) based on an event-by-event analysis of the different ions produced combined with an absolute target density determination. We are able to disentangle in detail the various proton ionization channels from mass-analyzed product ion signals in coincidence with the charge-analyzed projectile. In addition we are able to determine a complete set of cross sections for the ionization of these molecular targets by 20-150 keV protons including the total and partial cross sections and the direct-ionization and electron-capture cross sections.

  10. Photo-ionization cross-section of donor-related in (In,Ga)N/GaN core/shell under hydrostatic pressure and electric field effects

    NASA Astrophysics Data System (ADS)

    El Ghazi, Haddou; John Peter, A.

    2017-04-01

    Hydrogenic-like donor-impurity related self and induced polarizations, bending energy and photo-ionization cross section in spherical core/shell zinc blende (In,Ga)N/GaN are computed. Based on the variational approach and within effective-mass and one parabolic approximations, the calculations are made under finite potential barrier taking into account of the discontinuity of the effective-mass and the constant dielectric. The photo-ionization cross section is studied according to the photon incident energy considering the effects of hydrostatic pressure, applied electric field, structure's radius, impurity's position and indium composition in the core. It is obtained that the influences mentioned above lead to either blue shifts or redshifts of the resonant peak of the photo-ionization cross section spectrum. The unusual behavior related to the structure radius is discussed which is as a consequence of the finite potential confinement. We have shown that the photo-ionization cross section can be controlled with adjusting the internal and external factors. These properties can be useful for producing some device applications such as quantum dot infrared photodetectors.

  11. Absolute triple-differential cross sections for ionization-excitation of helium

    SciTech Connect

    Bartschat, K.; Bray, I.; Fursa, D. V.; Stelbovics, A. T.

    2007-08-15

    Triple-differential cross sections (TDCSs) for electron-impact ionization of He(1s{sup 2}){sup 1}S leading to He{sup +}(1s) are calculated using the highly accurate convergent close-coupling (CCC) method for incident projectile energies of 268.6 and 112.6 eV, with at least one of the outgoing electrons having an energy of 44 eV. These results are used to obtain absolute TDCSs from the recent experimental data [Bellm et al., Phys. Rev. A 75, 042704 (2007)] for TDCS ratios of ionization with no excitation to ionization with excitation resulting in He{sup +}(n=2,3,4). The TDCSs can be used as comparison benchmarks in future studies, and already allow us to test the accuracy of the TDCSs obtained from the hybrid distorted-wave+R-matrix (close-coupling) model, which was fairly successful in predicting the ratios, using CCC for n=1 and experimental results for n=2,3,4.

  12. Absolute cross sections for dissociative electron attachment to HCN and DCN

    SciTech Connect

    May, O.; Kubala, D.; Allan, M.

    2010-07-15

    Absolute partial cross sections for the formation of CN{sup -} in dissociative electron attachment to HCN and DCN have been measured using a time-of-flight ion spectrometer combined with a trochoidal electron monochromator to be 940pm{sup 2} for CN{sup -}/HCN and 340pm{sup 2} for CN{sup -}/DCN at peaks of the bands due to the {sup 2{Pi}}-shape resonance. The dissociative electron attachment bands were then recorded under higher resolution, 60 meV, with a trochoidal monochromator plus quadrupole mass filter combination and found to have a nearly vertical onset at the threshold energy and to peak at 1.85 eV. Broad structure was observed on the bands, assigned to formation of vibrationally excited CN{sup -}, from which the branching ratios could be determined to be 1,0.49, and 0.22 for the formation of CN{sup -} in the v=0,1, and 2 states, respectively. The results are compared to the recent multidimensional ab initio calculations of Chourou and Orel [Phys. Rev. A 80, 032709 (2009)].

  13. Measurements of mass attenuation coefficients and determination of photoionization cross sections at energies across the Li (i=1-3) edges of 66Dy

    NASA Astrophysics Data System (ADS)

    Kaur, Rajnish; Kumar, Anil; Osan, Janos; Czyzycki, M.; Karydas, A. G.; Puri, Sanjiv

    2017-07-01

    The absolute values of the mass attenuation coefficients have been measured at sixty two photon energies across the Li (i=1-3) sub-shell absorption edges of 66Dy covering the region 7.6-14.0 keV in order to investigate the influence of near-edge processes on the attenuation coefficients. The present measured attenuation coefficients are found to be higher by up to 10% than the theoretical values evaluated from the computer code XCOM (Berger et al., 2010) and the self-consistent Dirac-Hartree-Slater (DHS) model based values tabulated by Chantler (1995) over the energy region 7.6-14.0 keV, except at energies in vicinity (few eV) of the Li (i=1-3) sub-shell absorption edge energies where the measured values are significantly higher (up to 37%) than both the sets of theoretical values. Further, the Li (i=1-3) sub-shell photoionization cross sections, (σLiP)exp, deduced from the present measured mass attenuation coefficients are compared with the non-relativistic Hartree-Fock-Slater (HFS) model based values tabulated by Scofield (1973) and those evaluated from the theoretical total photoionization attenuation coefficients tabulated by Chantler (1995). The deduced (σLiP)exp(i=1-3) values are found to be in better agreement with those evaluated from the tabulations given by Chantler (1995) than the values given by Scofield (1973) over the energy region 7.8 - 14.0 keV included in this study. However, at photon energies up to few eV above the Li edges, the deduced (σLiP)exp(i=1-3) values are found to be significantly higher (up to 32%) than both the sets of theoretical values.

  14. Measurements of absolute M-subshell X-ray production cross sections of Th by electron impact

    NASA Astrophysics Data System (ADS)

    Moy, A.; Merlet, C.; Dugne, O.

    2014-08-01

    Measurements of absolute M-subshell X-ray production cross sections for element Th were made by electron impact for energies ranging from the ionization threshold up to 38 keV. Experimental data were obtained by measuring the X-ray intensity emitted from ultrathin Th films deposited onto self-supporting C backing films. The measurements were conducted with an electron microprobe using high-resolution wavelength dispersive spectrometers. Recorded intensities were converted into absolute X-ray production cross sections by means of atomic data and estimation of the number of primary electrons, target thickness, and detector efficiency. Our experimental X-ray production cross sections, the first to be reported for the M subshells of Th, are compared with X-ray production cross sections calculated with the mean of ionization cross sections obtained from the distorted-wave Born approximation. The Mα X-ray production cross section calculated is in excellent agreement with the measurements, allowing future use for standardless quantification in electron probe microanalysis.

  15. Absolute Rayleigh scattering cross sections of gases and freons of stratospheric interest in the visible and ultraviolet regions

    NASA Technical Reports Server (NTRS)

    SHARDANAND; Rao, A. D. P.

    1977-01-01

    The laboratory measurements of absolute Rayleigh scattering cross sections as a function wavelength are reported for gas molecules He, Ne, Ar, N2, H2, O2, CO2, CH4 and for vapors of most commonly used freons CCl2F2, CBrF3, CF4, and CHClf2. These cross sections are determined from the measurements of photon scattering at an angle of 54 deg 44 min which yield the absolute values independent of the value of normal depolarization ratios. The present results show that in the spectral range 6943-3638A deg, the values of the Rayleigh scattering cross section can be extrapolated from one wavelength to the other using 1/lambda (4) law without knowing the values of the polarizabilities. However, such an extrapolation can not be done in the region of shorter wavelengths.

  16. Absolute elastic differential electron scattering cross sections for He - A proposed calibration standard from 5 to 200 eV

    NASA Technical Reports Server (NTRS)

    Register, D. F.; Trajmar, S.; Srivastava, S. K.

    1980-01-01

    Absolute differential, integral, and momentum-transfer cross sections for electrons elastically scattered from helium are reported for the impact energy range of 5 to 200 eV. Angular distributions for elastically scattered electrons are measured in a crossed-beam geometry using a collimated, differentially pumped atomic-beam source which requires no effective-path-length correction. Below the first inelastic threshold the angular distributions were placed on an absolute scale by use of a phase-shift analysis. Above this threshold, the angular distributions from 10 to 140 deg were fitted using the phase-shift technique, and the resulting integral cross sections were normalized to a semiempirically derived integral elastic cross section. Depending on the impact energy, the data are estimated to be accurate to within 5 to 9%.

  17. Measurement of the absolute Raman cross section of the optical phonon in silicon

    NASA Astrophysics Data System (ADS)

    Aggarwal, R. L.; Farrar, L. W.; Saikin, S. K.; Aspuru-Guzik, A.; Stopa, M.; Polla, D. L.

    2011-04-01

    The absolute Raman cross section σ of the first-order 519 cm -1 optical phonon in silicon was measured using a small temperature-controlled blackbody for the signal calibration of the Raman system. Measurements were made with a 25-mil thick (001) silicon sample located in the focal plane of a 20-mm effective focal length (EFL) lens using 785-, 1064-, and 1535-nm CW pump lasers for the excitation of Raman scattering. The pump beam was polarized along the [100] axis of the silicon sample. Values of 1.0±0.2×10 -27, 3.6±0.7×10 -28, and 1.1±0.2×10 -29 cm 2 were determined for σ for 785-, 1064-, and 1535-nm excitation, respectively. The corresponding values of the Raman scattering efficiency S are 4.0±0.8×10 -6, 1.4±0.3×10 -6, and 4.4±0.8×10 -8 cm -1 sr -1.The values of the Raman polarizability |d| for 785-, 1064-, and 1535-nm excitation are 4.4±0.4×10 -15, 5.1±0.5×10 -15, and 1.9±0.2×10 -15 cm 2, respectively. The values of 4.4±0.4×10 -15 and 5.1±0.5×10 -15 cm 2 for |d| for 785- and 1064-nm excitation, respectively, are 1.3 and 2.0 times larger than the values of 3.5×10 -15 and 2.5×10 -15 cm 2 calculated by Wendel. The Raman polarizability |d| computed using the density functional theory in the long-wavelength limit is consistent with the general trend of the measured data and Wendel's model.

  18. Absolute cross sections for electronic excitation of pyrimidine by electron impact

    SciTech Connect

    Regeta, Khrystyna; Allan, Michael; Mašín, Zdeněk; Gorfinkiel, Jimena D.

    2016-01-14

    We measured differential cross sections for electron-impact electronic excitation of pyrimidine, both as a function of electron energy up to 18 eV, and of scattering angle up to 180°. The emphasis of the present work is on recording detailed excitation functions revealing resonances in the excitation process. The differential cross sections were summed to obtain integral cross sections. These are compared to results of R-matrix calculations, which successfully reproduce both the magnitude of the cross section and the major resonant features. Comparison of the experiment to the calculated contributions of different symmetries to the integral cross section permitted assignment of several features to specific core-excited resonances. Comparison of the resonant structure of pyrimidine with that of benzene revealed pronounced similarities and thus a dominant role of π–π{sup ∗} excited states and resonances. Electron energy loss spectra were measured as a preparation for the cross section measurements and vibrational structure was observed for some of the triplet states. A detailed analysis of the electronic excited states of pyrimidine is also presented.

  19. Absolute cross sections for electronic excitation of pyrimidine by electron impact

    NASA Astrophysics Data System (ADS)

    Regeta, Khrystyna; Allan, Michael; Mašín, Zdeněk; Gorfinkiel, Jimena D.

    2016-01-01

    We measured differential cross sections for electron-impact electronic excitation of pyrimidine, both as a function of electron energy up to 18 eV, and of scattering angle up to 180°. The emphasis of the present work is on recording detailed excitation functions revealing resonances in the excitation process. The differential cross sections were summed to obtain integral cross sections. These are compared to results of R-matrix calculations, which successfully reproduce both the magnitude of the cross section and the major resonant features. Comparison of the experiment to the calculated contributions of different symmetries to the integral cross section permitted assignment of several features to specific core-excited resonances. Comparison of the resonant structure of pyrimidine with that of benzene revealed pronounced similarities and thus a dominant role of π-π∗ excited states and resonances. Electron energy loss spectra were measured as a preparation for the cross section measurements and vibrational structure was observed for some of the triplet states. A detailed analysis of the electronic excited states of pyrimidine is also presented.

  20. Absolute measurement of the differential cross section for deuteron photodisintegration from 63 to 71 MeV

    SciTech Connect

    Debevec, P.T.; Harty, P.D.; Knott, J.E. ); Jenkins, D.A.; Jones, R.T. )

    1992-03-01

    The absolute differential cross section for the {sup 2}H({gamma},{ital p}){ital n} reaction has been measured using a large solid angle detector, with a tagged photon beam of mean energy 67 MeV. The data have been compared with nine different theoretical calculations of the cross section, which account for the data to varying degrees. Best agreement is obtained for models utilizing the nonrelativistic impulse approximation with a realistic nuclear potential, meson-exchange currents, and relativistic corrections.

  1. The recent absolute total np and pp cross section determinations: quality of data description and prediction of experimental observables

    SciTech Connect

    Laptev, Alexander B; Haight, Robert C; Arndt, Richard A; Briscoe, William J; Paris, Mark W; Strakovsky, Igor I; Workman, Ron L

    2010-01-01

    The absolute total cross sections for np and pp scattering below 1000 MeV are determined based on partial-wave analyses (PWAs) of nucleon-nucleon scattering data. These cross sections are compared with the most recent ENDF/B-VII.0 and JENDL-3.3 data files, and the Nijmegen PWA. Systematic deviations from the ENDF/B-VII.0 and JENDL-3.3 evaluations are found to exist in the low-energy region. Comparison of the np evaluation with the result of most recent np total and differential cross section measurements will be discussed. Results of those measurements were not used in the evaluation database. A comparison was done to check a quality of evaluation and its capabilities to predict experimental observables. Excellent agreement was found between the new experimental data and our PWA predictions.

  2. Absolute elastic differential electron scattering cross sections in the intermediate energy region. III - SF6 and UF6

    NASA Technical Reports Server (NTRS)

    Srivastava, S. K.; Trajmar, S.; Chutjian, A.; Williams, W.

    1976-01-01

    A recently developed technique has been used to measure the ratios of elastic differential electron scattering cross sections (DCS) for SF6 and UF6 to those of He at electron impact energies of 5, 10, 15, 20, 30, 40, 50, 60, and 75 eV and at scattering angles of 20 to 135 deg. In order to obtain the absolute values of DCS from these ratios, He DCS of McConkey and Preston have been employed in the 20 to 90 deg range. At angles in the 90 to 135 deg range the recently determined cross sections of Srivastava and Trajmar have been utilized. From these DCS, elastic integral and momentum transfer cross sections have been obtained.

  3. Absolute Cross Sections for Proton Induced Reactions on 147,149Sm Below the Coulomb Barrier

    NASA Astrophysics Data System (ADS)

    Gheorghe, I.; Filipescu, D.; Glodariu, T.; Bucurescu, D.; Cata-Danil, I.; Cata-Danil, G.; Deleanu, D.; Ghita, D.; Ivascu, M.; Lica, R.; Marginean, N.; Marginean, R.; Mihai, C.; Negret, A.; Sava, T.; Stroe, L.; Toma, S.; Sima, O.; Sin, M.

    2014-05-01

    Cross sections for 147,149Sm(p,n)147,149Eu and 147,149Sm(p, γ)148,150Eu were measured using the activation method. The results are compared to the predictions of the Hauser-Feshbach statistical model. Different γ-ray strength functions have been tested against the experimental values. In the case of 150Eu, in order to reproduce the experimental isomeric population cross sections, various scenarios for unknown branching ratios of certain discrete states have been discussed. The results provide constraints for the optical model parameters dedicated to this insufficiently known area of isotopes. Such cross sections for (p, γ) reactions at energies below the Coulomb barrier are valuable for p-process nucleosynthesis calculations.

  4. Absolute Measurements of Drell-Yan Cross Sections in 800 GeV pN Collisions

    NASA Astrophysics Data System (ADS)

    Webb, Jason

    2002-04-01

    The production of massive lepton pairs in proton-nucleon collisions is an important probe of the anti-quark distributions in the nucleon. FNAL E866/NuSea has measured the ratio σ_pd/σ_pp for proton induced dimuon production, which provides important constraints on the ratio of anti-down to anti-up quarks as a function of Björken-x. Absolute measurements of the proton-proton and proton-deuteron cross sections provide complementary information on bard(x)+baru(x) and baru(x). Results for both the cross section ratio and absolute measurements are presented and compared with NLO calculations based on current parton distribution functions.

  5. Absolute cross sections for electronic excitations of cytosine by low energy electron impact

    PubMed Central

    Bazin, M.; Michaud, M.; Sanche, L.

    2013-01-01

    The absolute cross sections (CS) for electronic excitations of cytosine by electron impact between 5 and 18 eV were measured by electron-energy loss (EEL) spectroscopy of the molecule deposited at low coverage on an inert Ar substrate. The lowest EEL features found at 3.55 and 4.02 eV are ascribed to transitions from the ground state to the two lowest triplet 1 3A′(π→π*) and 2 3A′(π→π*) valence states of the molecule. Their energy dependent CS exhibit essentially a common maximum at about 6 eV with a value of 1.84 × 10−17 cm2 for the former and 4.94 × 10−17 cm2 for the latter. In contrast, the CS for the next EEL feature at 4.65 eV, which is ascribed to the optically allowed transition to the 2 1A′(π→π*) valence state, shows only a steep rise to about 1.04 × 10−16 cm2 followed by a monotonous decrease with the incident electron energy. The higher EEL features at 5.39, 6.18, 6.83, and 7.55 eV are assigned to the excitations of the 3 3, 1A′(π→π*), 4 1A′(π→π*), 5 1A′(π→π*), and 6 1A′(π→π*) valence states, respectively. The CS for the 3 3, 1A′ and 4 1A′ states exhibit a common enhancement at about 10 eV superimposed on a more or less a steep rise, reaching respectively a maximum of 1.27 and 1.79 × 10−16 cm2, followed by a monotonous decrease. This latter enhancement and the maximum seen at about 6 eV in the lowest triplet states correspond to the core-excited electron resonances that have been found by dissociative electron attachment experiments with cytosine in the gas phase. The weak EEL feature found at 5.01 eV with a maximum CS of 3.8 × 10−18 cm2 near its excitation threshold is attributed to transitions from the ground state to the 1 3, 1A″(n→π*) states. The monotonous rise of the EEL signal above 8 eV is attributed to the ionization of the molecule. It is partitioned into four excitation energy regions at about 8.55, 9.21, 9.83, and 11.53 eV, which correspond closely to the ionization energies of

  6. Absolute cross sections for vibrational excitations of cytosine by low energy electron impact

    PubMed Central

    Michaud, M.; Bazin, M.; Sanche, L.

    2013-01-01

    The absolute cross sections (CSs) for vibrational excitations of cytosine by electron impact between 0.5 and 18 eV were measured by electron-energy loss (EEL) spectroscopy of the molecule deposited at monolayer coverage on an inert Ar substrate. The vibrational energies compare to those that have been reported from IR spectroscopy of cytosine isolated in Ar matrix, IR and Raman spectra of poly-crystalline cytosine, and ab initio calculation. The CSs for the various H bending modes at 142 and 160 meV are both rising from their energy threshold up to 1.7 and 2.1 × 10−17 cm2 at about 4 eV, respectively, and then decrease moderately while maintaining some intensity at 18 eV. The latter trend is displayed as well for the CS assigned to the NH2 scissor along with bending of all H at 179 meV. This overall behavior in electron-molecule collision is attributed to direct processes such as the dipole, quadrupole, and polarization contributions, etc. of the interaction of the incident electron with a molecule. The CSs for the ring deformation at 61 meV, the ring deformation with N-H symmetric wag at 77 meV, and the ring deformations with symmetric bending of all H at 119 meV exhibit common enhancement maxima at 1.5, 3.5, and 5.5 eV followed by a broad hump at about 12 eV, which are superimposed on the contribution due to the direct processes. At 3.5 eV, the CS values for the 61-, 77-, and 119-meV modes reach 4.0, 3.0, and 4.5 × 10−17 cm2, respectively. The CS for the C-C and C-O stretches at 202 meV, which dominates in the intermediate EEL region, rises sharply until 1.5 eV, reaches its maximum of 5.7 × 10−17 cm2 at 3.5 eV and then decreases toward 18 eV. The present vibrational enhancements, correspond to the features found around 1.5 and 4.5 eV in electron transmission spectroscopy (ETS) and those lying within 1.5–2.1 eV, 5.2–6.8 eV, and 9.5–10.9 eV range in dissociative electron attachment (DEA) experiments with cytosine in gas phase. While the ETS features

  7. Supplementary absolute differential cross sections for the excitation of atomic hydrogen's n=3 and 4 levels by electron impact

    SciTech Connect

    Sweeney, Christopher J.; Shyn, Tong W.; Grafe, Alan

    2004-05-01

    We have conducted measurements of absolute differential cross sections for the excitation of hydrogen atoms to their n=3(3S+3P+3D) and 4(4S+4P+4D+4F) levels. A modulated, crossed-beam method was employed, and the impact energies were 40 and 60 eV. Comparison of our results with those of others is quite favorable.

  8. Measurement of the absolute differential cross section of proton–proton elastic scattering at small angles

    SciTech Connect

    Mchedlishvili, D.; Chiladze, D.; Dymov, S.; Bagdasarian, Z.; Barsov, S.; Gebel, R.; Gou, B.; Hartmann, M.; Kacharava, A.; Keshelashvili, I.; Khoukaz, A.; Kulessa, P.; Kulikov, A.; Lehrach, A.; Lomidze, N.; Lorentz, B.; Maier, R.; Macharashvili, G.; Merzliakov, S.; Mikirtychyants, S.; Nioradze, M.; Ohm, H.; Prasuhn, D.; Rathmann, F.; Serdyuk, V.; Schroer, D.; Shmakova, V.; Stassen, R.; Stein, H. J.; Stockhorst, H.; Strakovsky, I. I.; Stroher, H.; Tabidze, M.; Taschner, A.; Trusov, S.; Tsirkov, D.; Uzikov, Yu.; Valdau, Yu.; Wilkin, C.; Workman, R. L.; Wustner, P.

    2016-02-03

    The differential cross section for proton-proton elastic scattering has been measured at a beam kinetic energy of 1.0 GeV and in 200 MeV steps from 1.6 to 2.8 GeV for centre-of-mass angles in the range from 12°-16° to 25°-30°, depending on the energy. A precision in the overall normalisation of typically 3% was achieved by studying the energy losses of the circulating beam of the COSY storage ring as it passed repeatedly through the windowless hydrogen target of the ANKE magnetic spectrometer. It is shown that the data have a significant impact upon the results of a partial wave analysis. Furthermore, after extrapolating the differential cross sections to the forward direction, the results are broadly compatible with the predictions of forward dispersion relations.

  9. Measurement of the absolute differential cross section of proton–proton elastic scattering at small angles

    DOE PAGES

    Mchedlishvili, D.; Chiladze, D.; Dymov, S.; ...

    2016-02-03

    The differential cross section for proton-proton elastic scattering has been measured at a beam kinetic energy of 1.0 GeV and in 200 MeV steps from 1.6 to 2.8 GeV for centre-of-mass angles in the range from 12°-16° to 25°-30°, depending on the energy. A precision in the overall normalisation of typically 3% was achieved by studying the energy losses of the circulating beam of the COSY storage ring as it passed repeatedly through the windowless hydrogen target of the ANKE magnetic spectrometer. It is shown that the data have a significant impact upon the results of a partial wave analysis.more » Furthermore, after extrapolating the differential cross sections to the forward direction, the results are broadly compatible with the predictions of forward dispersion relations.« less

  10. Absolute cross section for electron-impact ionization of He (1 s 2 s 3S)

    NASA Astrophysics Data System (ADS)

    Génévriez, Matthieu; Jureta, Jozo J.; Defrance, Pierre; Urbain, Xavier

    2017-07-01

    We present an experimental determination of the electron-impact ionization cross section of the 1 s 2 s 3S state of helium, for which there is a serious long-lasting discrepancy between theory and experiment. A technique for the production of a fast, intense beam of helium in the 1 s 2 s 3S state only has been developed for this purpose, based on photodetachment of the He- anion. The cross section is measured using the animated crossed beam technique. The present results are much lower than the experimental data of Dixon et al. [J. Phys. B 9, 2617 (1976), 10.1088/0022-3700/9/15/013] and are in excellent agreement with the calculation of Fursa and Bray [J. Phys. B 36, 1663 (2003), 10.1088/0953-4075/36/8/317].

  11. Dissociative Recombination and Excitation of CH{sup {plus}} {sub 5} : Absolute Cross Sections and Branching Fractions

    SciTech Connect

    Semaniak, J.; Larson, A.; Le Padellec, A.; Stroemholm, C.; Larsson, M.; Rosen, S.; Peverall, R.; Danared, H.; Djuric, N.; Dunn, G.H.; Datz, S.

    1998-05-01

    The heavy-ion storage ring CRYRING was used to measure the absolute dissociative recombination and dissociative excitation cross sections for collision energies below 50 eV. Deduced thermal rates coefficients are consistent with previous beams data but are lower by a factor of 3 than the rates measured by means of the flowing afterglow Langmuir probe technique. A resonant structure in dissociative recombination cross section was found at 9 eV. We have determined the branching fractions in DR of CH{sup {plus}} {sub 5} below 0.2 eV. The branching is dominated by three-body CH{sub 3} + H + H and CH{sub 2} + H{sub 2} + H dissociation channels, which occur with branching ratios of {approx}0.7 and {approx}0.2, respectively; thus methane is a minor species among dissociation products. Both the measured absolute cross sections and branching in dissociative recombination of CH{sup {plus}} {sub 5} can have important implications for the models of dense interstellar clouds and abundance of CH{sub 2}, CH{sub 3} and CH{sub 4} in these media. {copyright} {ital {copyright} 1998.} {ital The American Astronomical Society}

  12. Absolute Charge Exchange Cross Sections for ^3He^2+ Collisions with ^4He and H_2

    NASA Astrophysics Data System (ADS)

    Mawhorter, R. J.; Greenwood, J.; Smith, S. J.; Chutjian, A.

    2002-05-01

    The JPL charge exchange beam-line(J.B. Greenwood, et al., Phys. Rev A 63), 062707 (2001) was modified to increase the forward acceptance angle and enable the measurement of total charge-exchange cross sections for slow, light, highly-charged ion collisions with neutral targets(R. E. Olson and M. Kimura, J. Phys. B 15), 4231 (1982). Data are presented for single charge exchange cross sections for ^3He^2+ nuclei scattered by ^4He and H2 in the energy range 0.33-4.67 keV/amu. For both targets there is good agreement with Kusakabe, et al.(T. Kusakabe, et al., J. Phys. Soc. Japan 59), 1218 (1990). Angular collection is studied by a comparison with differential measurements(D. Bordenave-Montesquieu and R. Dagnac, J. Phys. B 27), 543 (1994), as well as with earlier JPL results(J.B. Greenwood, et al., Ap. J. 533), L175 (2000), ibid. 529, 605 (2000) using heavier projectiles and targets. This work was carried out at JPL/Caltech, and was supported through contract with NASA. RJM thanks the NRC for a Senior Associateship at JPL.

  13. Absolute Charge Transfer and Fragmentation Cross Sections in He{sup 2+}-C{sub 60} Collisions

    SciTech Connect

    Rentenier, A.; Moretto-Capelle, P.; Bordenave-Montesquieu, D.; Bordenave-Montesquieu, A.; Ruiz, L. F.; Diaz-Tendero, S.; Alcami, M.; Martin, F.; Zarour, B.; Hanssen, J.; Hervieux, P.-A.; Politis, M. F.

    2008-05-09

    We have determined absolute charge transfer and fragmentation cross sections in He{sup 2+}+C{sub 60} collisions in the impact-energy range 0.1-250 keV by using a combined experimental and theoretical approach. We have found that the cross sections for the formation of He{sup +} and He{sup 0} are comparable in magnitude, which cannot be explained by the sole contribution of pure single and double electron capture but also by contribution of transfer-ionization processes that are important even at low impact energies. The results show that multifragmentation is important only at impact energies larger than 40 keV; at lower energies, sequential C{sub 2} evaporation is the dominant process.

  14. Absolute K-shell ionization cross sections and L{alpha} and L{beta}{sub 1} x-ray production cross sections of Ga and As by 1.5-39-keV electrons

    SciTech Connect

    Merlet, C.; Llovet, X.; Fernandez-Varea, J. M.

    2006-06-15

    Absolute K-shell ionization and L{alpha} and L{beta}{sub 1} x-ray production cross sections for Ga and As have been measured for incident electrons in the energy range from 1.5 to 39 keV. The cross sections were deduced from K{alpha}, L{alpha}, and L{beta}{sub 1} x-ray intensities emitted from ultrathin GaAs samples deposited onto self-supporting carbon films. The x-ray intensities were measured on an electron microprobe equipped with several wavelength-dispersive spectrometers and were converted into absolute cross sections by using estimated values of the target thickness, spectrometer efficiency, and number of incident electrons. Experimental results are compared with cross sections calculated from the plane-wave and distorted-wave Born approximations, the relativistic binary-encounter-Bethe model, the results of two widely used simple analytical formulas, and, whenever possible, experimental data from the literature.

  15. Absolute cross sections for electronic excitation of condensed tetrahydrofuran (THF) by 11-16 eV electrons.

    PubMed

    Lemelin, V; Bass, A D; Cloutier, P; Sanche, L

    2016-11-07

    Absolute cross section (CS) data on the interaction of low energy electrons with DNA and its molecular constituents are required as input parameters in Monte-Carlo type simulations, for several radiobiological applications. Previously [V. Lemelin et al., J. Chem. Phys. 144, 074701 (2016)], we measured absolute vibrational CSs for low-energy electron scattering from condensed tetrahydrofuran, a convenient surrogate for the deoxyribose. Here we report absolute electronic CSs for energy losses of between 6 and 11.5 eV, by electrons with energies between 11 and 16 eV. The variation of these CSs with incident electron energy shows no evidence of transient anion states, consistent with theoretical and other experimental results, indicating that initial electron capture leading to DNA strand breaks occurs primarily on DNA bases or the phosphate group.

  16. Absolute cross sections for electronic excitation of condensed tetrahydrofuran (THF) by 11-16 eV electrons

    NASA Astrophysics Data System (ADS)

    Lemelin, V.; Bass, A. D.; Cloutier, P.; Sanche, L.

    2016-11-01

    Absolute cross section (CS) data on the interaction of low energy electrons with DNA and its molecular constituents are required as input parameters in Monte-Carlo type simulations, for several radiobiological applications. Previously [V. Lemelin et al., J. Chem. Phys. 144, 074701 (2016)], we measured absolute vibrational CSs for low-energy electron scattering from condensed tetrahydrofuran, a convenient surrogate for the deoxyribose. Here we report absolute electronic CSs for energy losses of between 6 and 11.5 eV, by electrons with energies between 11 and 16 eV. The variation of these CSs with incident electron energy shows no evidence of transient anion states, consistent with theoretical and other experimental results, indicating that initial electron capture leading to DNA strand breaks occurs primarily on DNA bases or the phosphate group.

  17. Absolute cross sections for electronic excitation of condensed tetrahydrofuran (THF) by 11–16 eV electrons

    PubMed Central

    Lemelin, V.; Bass, A. D.; Cloutier, P.; Sanche, L.

    2016-01-01

    Absolute cross section (CS) data on the interaction of low energy electrons with DNA and its molecular constituents are required as input parameters in Monte-Carlo type simulations, for several radiobiological applications. Previously [V. Lemelin et al., J. Chem. Phys. 144, 074701 (2016)], we measured absolute vibrational CSs for low-energy electron scattering from condensed tetrahydrofuran, a convenient surrogate for the deoxyribose. Here we report absolute electronic CSs for energy losses of between 6 and 11.5 eV, by electrons with energies between 11 and 16 eV. The variation of these CSs with incident electron energy shows no evidence of transient anion states, consistent with theoretical and other experimental results, indicating that initial electron capture leading to DNA strand breaks occurs primarily on DNA bases or the phosphate group. PMID:27825202

  18. Photoabsorption and photoionization cross sections of NH3, PH3, H2S, C2H2, and C2H4 in the VUV region

    NASA Technical Reports Server (NTRS)

    Xia, T. J.; Chien, T. S.; Wu, C. Y. Robert; Judge, D. L.

    1991-01-01

    Using synchrotron radiation as a continuum light source, the photoabsorption and photoionization cross sections of NH3, PH3, H2S, C2H2, and C2H4 have been measured from their respective ionization thresholds to 1060 A. The vibrational constants associated with the nu(2) totally symmetric, out-of-plane bending vibration of the ground electronic state of PH3(+) have been obtained. The cross sections and quantum yields for producing neutral products through photoexcitation of these molecules in the given spectral regions have also been determined. In the present work, autoionization processes were found to be less important than dissociation and predissociation processes in NH3, PH3, and C2H4. Several experimental techniques have been employed in order to examine the various possible systematic errors critically.

  19. Resonances in the Photoionization Cross Sections of Atomic Nitrogen Shape the Far-ultraviolet Spectrum of the Bright Star in 47 Tucanae

    NASA Astrophysics Data System (ADS)

    Dixon, William V.; Chayer, Pierre

    2013-08-01

    The far-ultraviolet spectrum of the Bright Star (B8 III) in 47 Tuc (NGC 104) shows a remarkable pattern: it is well fit by local thermodynamic equilibrium models at wavelengths longer than Lyβ, but at shorter wavelengths it is fainter than the models by a factor of two. A spectrum of this star obtained with the Far Ultraviolet Spectroscopic Explorer shows broad absorption troughs with sharp edges at 995 and 1010 Å and a deep absorption feature at 1072 Å none of which are predicted by the models. We find that these features are caused by resonances in the photoionization cross sections of the first and second excited states of atomic nitrogen (2s 2 2p 3 2 D 0 and 2 P 0). Using cross sections from the Opacity Project, we can reproduce these features, but only if we use the cross sections at their full resolution, rather than the resonance-averaged cross sections usually employed to model stellar atmospheres. These resonances are strongest in stellar atmospheres with enhanced nitrogen and depleted carbon abundances, a pattern typical of post-asymptotic giant branch stars.

  20. RESONANCES IN THE PHOTOIONIZATION CROSS SECTIONS OF ATOMIC NITROGEN SHAPE THE FAR-ULTRAVIOLET SPECTRUM OF THE BRIGHT STAR IN 47 TUCANAE

    SciTech Connect

    Dixon, William V.; Chayer, Pierre E-mail: chayer@stsci.edu

    2013-08-10

    The far-ultraviolet spectrum of the Bright Star (B8 III) in 47 Tuc (NGC 104) shows a remarkable pattern: it is well fit by local thermodynamic equilibrium models at wavelengths longer than Ly{beta}, but at shorter wavelengths it is fainter than the models by a factor of two. A spectrum of this star obtained with the Far Ultraviolet Spectroscopic Explorer shows broad absorption troughs with sharp edges at 995 and 1010 A and a deep absorption feature at 1072 A; none of which are predicted by the models. We find that these features are caused by resonances in the photoionization cross sections of the first and second excited states of atomic nitrogen (2s {sup 2} 2p {sup 3} {sup 2} D {sup 0} and {sup 2} P {sup 0}). Using cross sections from the Opacity Project, we can reproduce these features, but only if we use the cross sections at their full resolution, rather than the resonance-averaged cross sections usually employed to model stellar atmospheres. These resonances are strongest in stellar atmospheres with enhanced nitrogen and depleted carbon abundances, a pattern typical of post-asymptotic giant branch stars.

  1. Absolute cross sections of the 86Sr(α,n)89Zr reaction at energies of astrophysical interest

    NASA Astrophysics Data System (ADS)

    Oprea, Andreea; Glodariu, Tudor; Filipescu, Dan; Gheorghe, Ioana; Mitu, Andreea; Boromiza, Marian; Bucurescu, Dorel; Costache, Cristian; Cata-Danil, Irina; Florea, Nicoleta; Ghita, Dan Gabriel; Ionescu, Alina; Marginean, Nicolae; Marginean, Raluca; Mihai, Constantin; Mihai, Radu; Negret, Alexandru; Nita, Cristina; Olacel, Adina; Pascu, Sorin; Sotty, Cristophe; Suvaila, Rares; Stan, Lucian; Stroe, Lucian; Serban, Andreea; Stiru, Irina; Toma, Sebastian; Turturica, Andrei; Ujeniuc, Sorin

    2017-09-01

    Absolute cross sections for the 86Sr(α,n)89Zr reaction at energies close to the Gamow window are reported. Three thin SrF2 targets were irradiated using the 9 MV Tandem facility in IFIN-HH Bucharest that delivered α beams for the activation process. Two high-purity Germanium detectors were used to measure the induced activity of 89Zr in a low background environment. The experimental results are in very good agreement with Hauser-Feshbach statistical model calculations performed with the TALYS code.

  2. Measurement of the absolute vμ-CCQE cross section at the SciBooNE experiment

    SciTech Connect

    Aunion, Jose Luis Alcaraz

    2010-07-01

    This thesis presents the measurement of the charged current quasi-elastic (CCQE) neutrino-nucleon cross section at neutrino energies around 1 GeV. This measurement has two main physical motivations. On one hand, the neutrino-nucleon interactions at few GeV is a region where existing old data are sparse and with low statistics. The current measurement populates low energy regions with higher statistics and precision than previous experiments. On the other hand, the CCQE interaction is the most useful interaction in neutrino oscillation experiments. The CCQE channel is used to measure the initial and final neutrino fluxes in order to determine the neutrino fraction that disappeared. The neutrino oscillation experiments work at low neutrino energies, so precise measurement of CCQE interactions are essential for flux measurements. The main goal of this thesis is to measure the CCQE absolute neutrino cross section from the SciBooNE data. The SciBar Booster Neutrino Experiment (SciBooNE) is a neutrino and anti-neutrino scattering off experiment. The neutrino energy spectrum works at energies around 1 GeV. SciBooNE was running from June 8th 2007 to August 18th 2008. In that period, the experiment collected a total of 2.65 x 1020 protons on target (POT). This thesis has used full data collection in neutrino mode 0.99 x 1020 POT. A CCQE selection cut has been performed, achieving around 70% pure CCQE sample. A fit method has been exclusively developed to determine the absolute CCQE cross section, presenting results in a neutrino energy range from 0.2 to 2 GeV. The results are compatible with the NEUT predictions. The SciBooNE measurement has been compared with both Carbon (MiniBoonE) and deuterium (ANL and BNL) target experiments, showing a good agreement in both cases.

  3. Photoionization cross sections of H2(+) and H2 with complex Gaussian-type basis functions optimized for the frequency-dependent polarizabilities.

    PubMed

    Morita, Masato; Yabushita, Satoshi

    2008-11-15

    Within the framework of the complex basis function method, the photoionization cross sections of H(2)(+) and H(2) were calculated based on the variational principle for the frequency-dependent polarizabilities. In these calculations, complex orbital exponents of Gaussian-type basis functions for the final state continuum wavefunctions were fully optimized for each photon energy with the numerical Newton-Raphson method. In most cases, the use of only one or two complex Gaussian-type basis functions was enough to obtain excellent agreement with previous high precision calculations and available experimental results. However, there were a few cases, in which the use of complex basis functions having various angular momentum quantum numbers was crucial to obtain the accurate results. The behavior of the complex orbital exponents as a function of photon energy was discussed in relation to the scaling relation and the effective charge for photoelectron. The success of this method implies the effectiveness of the optimization of orbital exponents to reduce the number of basis functions and shows the possibility to calculate photoionization cross sections of general molecules using only Gaussian-type basis functions.

  4. Multiconfigurational Hartree-Fock close-coupling ansatz: Application to the argon photoionization cross section and delays

    NASA Astrophysics Data System (ADS)

    Carette, T.; Dahlström, J. M.; Argenti, L.; Lindroth, E.

    2013-02-01

    We present a robust, ab initio method for addressing atom-light interactions and apply it to photoionization of argon. We use a close-coupling ansatz constructed on a multiconfigurational Hartree-Fock description of localized states and B-spline expansions of the electron radial wave functions. In this implementation, the general many-electron problem can be tackled thanks to the use of the atsp2k libraries [C. Froese Fischer , Comput. Phys. Commun.CPHCBZ0010-465510.1016/j.cpc.2007.01.006 176, 559 (2007)]. In the present contribution, we combine this method with exterior complex scaling, thereby allowing for the computation of the complex partial amplitudes that encode the whole dynamics of the photoionization process. The method is validated on the 3s3p6np series of resonances converging to the 3s extraction. Then, it is used for computing the energy dependent differential atomic delay between 3p and 3s photoemission, and agreement is found with the measurements of Guénot [Phys. Rev. APLRAAN1050-294710.1103/PhysRevA.85.053424 85, 053424 (2012)]. The effect of the presence of resonances in the one-photon spectrum on photoionization delay measurements is studied.

  5. Photoionization of the Buckminsterfullerene Cation.

    PubMed

    Douix, Suzie; Duflot, Denis; Cubaynes, Denis; Bizau, Jean-Marc; Giuliani, Alexandre

    2017-01-05

    Photoionization of a buckminsterfullerene ion is investigated using an ion trap and a merged beam setup coupled to synchrotron radiation beamlines and compared to theoretical calculations. Absolute measurements derived from the ion trap experiment allow discrepancies concerning the photoionization cross section of C60(+) to be solved.

  6. Absolute Total Cross Section Measurements for Electron Scattering on GeH4 and SiH4 Molecules

    NASA Astrophysics Data System (ADS)

    Zejko, Pawel. Mo.; Kasperski, Grzegorz; Szmytkowski, Czeslaw

    1996-10-01

    We have measured absolute grand total electron--scattering cross section for GeH4 and SiH4 molecules in the energy range of 0.75--250 eV and 0.6--250 eV, respectively, using the linear transmission experimental setup(A.M. Krzysztofowicz and Cz. Szmytkowski 1995 J. Phys. B 28) 1593. The general character of both obtained total cross section (TCS) functions is similar. For germane TCS dramatically increases from 12× 10-20 m^2 at 0.8 eV up to nearly 59× 10-20 m^2 at the 3.8 eV maximum. For silane the maximum (57× 10-20 m^2) is localized near 2.9 eV. These structures are partly attributable to the existence of short-lived negative-ion resonant states. From 10 eV to the highest applied energy TCS' decrease monotonically with increasing impact energy E, and above 50 eV the total cross sections change like E-0.5. None low-energy e^--GeH4 experiment is available for comparison. Above 75 eV our results are in good agreement with the recent intermediate-energy TCS measurements of Karwasz(G.P. Karwasz 1995 J. Phys. B 28) 1301 and with calculations of Baluja et al(K.L. Baluja et al) 1992 Europhys. Lett. 17 139. There is also reasonably agreement of present e^--SiH4 data with available experimental results.

  7. Absolute total electron scattering cross sections for N/sub 2/ between 0. 5 and 50 eV

    SciTech Connect

    Kennerly, R.E.

    1980-06-01

    Absolute total electron scattering cross sections for N/sub 2/ from 0.5 to 50 eV have been measured with an estimated uncertainty of +- 3% using a transmission time-of-flight method previously described. The results are compared to previous experimental results and to recent calculations. The positions of the /sup 2/Pi/sub g/ resonance peaks were determined with much greater accuracy ( +- 15 meV) than in previous transmission measurements. The structure reported by Golden (1966) below the /sup 2/Pi/sub g/ resonance was clearly not present, indicating that, if real, these features are not a property of the N/sub 2/ ground vibronic state. The shape resonance predicted at 11 eV by Dill and Dehmer (1977) was not seen, perhaps because it was too weakly manifested in the total cross section. A weak broad band centered at 25 eV may be interpreted as being due to a sigma/sub u/ shape resonance as predicted by Dehmer, Siegel, Welch, and Dill.

  8. Absolute Charge Exchange Cross Sections for O^5+, O^6+, and O^7+ Collisions with CO and CO2

    NASA Astrophysics Data System (ADS)

    Mawhorter, Richard; Djuric, Nada; Macaskill, John; Smith, Steven J.; Chutjian, Ara; Williams, Ian D.

    2005-05-01

    Motivated by ongoing EUV and X-ray studies of comets, we have continued our experimental investigations of absolute charge exchange cross sections for highly-charged ions present in the solar wind incident on cometary gases. These are the first measurements on the JPL charge exchange beam-line using a new LabView data acquisition system combined with a larger gas cell exit aperture. Data for O^5+ & O^7+ on CO2 agree with earlier measurements [1], and are included in these new results for O^5+, O^6+, and O^7+ on CO and CO2. The ion beam accelerating potential was 7 kV, which yields ion velocities consistent with the fast component of the solar wind. Agreement with earlier, smaller exit aperture measurements is also significant in demonstrating an independence from angular collection issues for these fast, heavy ions and targets. This was verified by studying collection angle-cross section effects for slow ^3He^2+ ions on He and H2. This work was carried out at JPL/Caltech, and was supported through contract with NASA. N.Djuric also acknowledges support through the NASA-NRC program. [1] J.B. Greenwood, et al., Phys. Rev A 63, 062707 (2001).

  9. Using DNA origami nanostructures to determine absolute cross sections for UV photon-induced DNA strand breakage.

    PubMed

    Vogel, Stefanie; Rackwitz, Jenny; Schürman, Robin; Prinz, Julia; Milosavljević, Aleksandar R; Réfrégiers, Matthieu; Giuliani, Alexandre; Bald, Ilko

    2015-11-19

    We have characterized ultraviolet (UV) photon-induced DNA strand break processes by determination of absolute cross sections for photoabsorption and for sequence-specific DNA single strand breakage induced by photons in an energy range from 6.50 to 8.94 eV. These represent the lowest-energy photons able to induce DNA strand breaks. Oligonucleotide targets are immobilized on a UV transparent substrate in controlled quantities through attachment to DNA origami templates. Photon-induced dissociation of single DNA strands is visualized and quantified using atomic force microscopy. The obtained quantum yields for strand breakage vary between 0.06 and 0.5, indicating highly efficient DNA strand breakage by UV photons, which is clearly dependent on the photon energy. Above the ionization threshold strand breakage becomes clearly the dominant form of DNA radiation damage, which is then also dependent on the nucleotide sequence.

  10. Electron-recoil ion and recoil ion-projectile coincidence techniques applied to obtain absolute partial collision cross sections.

    PubMed

    Wolff, W; de Souza, Ihani J; Tavares, André C; de Oliveira, G F S; Luna, H

    2012-12-01

    We present in detail an alternative experimental set-up and data analysis, based on the electron-recoil ion and recoil ion-projectile coincidence techniques, that enable the measurement of partial pure ionization and partial charge exchange cross sections for an effusive gas jet set-up, where the absolute target density and recoil ion efficiency cannot be measured directly. The method is applied to the ionization of helium atoms due to collision with partially stripped C(3 +) projectiles. In order to check the method, the results are compared to data available in the literature where the target density and recoil ion detection efficiency were measured directly. The pure ionization channel is compared to the electron capture channel.

  11. Absolute vibrational cross sections for 1-19 eV electron scattering from condensed tetrahydrofuran (THF)

    NASA Astrophysics Data System (ADS)

    Lemelin, V.; Bass, A. D.; Cloutier, P.; Sanche, L.

    2016-02-01

    Absolute cross sections (CSs) for vibrational excitation by 1-19 eV electrons impacting on condensed tetrahydrofuran (THF) were measured with a high-resolution electron energy loss spectrometer. Experiments were performed under ultra-high vacuum (3 × 10-11 Torr) at a temperature of about 20 K. The magnitudes of the vibrational CSs lie within the 10-17 cm2 range. Features observed near 4.5, 9.5, and 12.5 eV in the incident energy dependence of the CSs were compared to the results of theoretical calculations and other experiments on gas and solid-phase THF. These three resonances are attributed to the formation of shape or core-excited shape resonances. Another maximum observed around 2.5 eV is not found in the calculations but has been observed in gas-phase studies; it is attributed to the formation of a shape resonance.

  12. Absolute differential cross sections for the elastic scattering of electrons from atomic hydrogen at low incident energies

    NASA Astrophysics Data System (ADS)

    James, Kenneth; Leonard, Linda; Proctor, Stephanie; Childers, J. G.; Khakoo, Murtadha A.

    2003-05-01

    Absolute differential cross sections for electrons elastically scattered from atomic hydrogen have been measured at low incident energies. The measurements were facilitated by the moveable nozzle source recently developed in our lab. Data taken at the incident energies of 20 eV, 40 eV, and 100 eV, and spanning the angular range of 10^rc to 120^rc will be presented. The results will be compared to the earlier measurements of Williams(Joseph Callaway and J. F. Williams, Phys. Rev. A) 12, 2312 (1975), J. F. Williams, J. Phys. B 8, 2191 (1975) and Shyn(T. W. Shyn and S. Y. Cho, Phys. Rev. A) 40, 1315 (1989), T. W. Shyn and Alan Grafe, Phys. Rev. A 46, 2949 (1992), and the theoretical calculations of Bray(Igor Bray, Phys. Rev. A) 46, 6995 (1992). Funded by the National Science Foundation under Grant # NSF-RUI-PHY-0096808.

  13. Absolute vibrational cross sections for 1–19 eV electron scattering from condensed tetrahydrofuran (THF)

    PubMed Central

    Lemelin, V.; Bass, A. D.; Cloutier, P.; Sanche, L.

    2016-01-01

    Absolute cross sections (CSs) for vibrational excitation by 1–19 eV electrons impacting on condensed tetrahydrofuran (THF) were measured with a high-resolution electron energy loss spectrometer. Experiments were performed under ultra-high vacuum (3 × 10−11 Torr) at a temperature of about 20 K. The magnitudes of the vibrational CSs lie within the 10−17 cm2 range. Features observed near 4.5, 9.5, and 12.5 eV in the incident energy dependence of the CSs were compared to the results of theoretical calculations and other experiments on gas and solid-phase THF. These three resonances are attributed to the formation of shape or core-excited shape resonances. Another maximum observed around 2.5 eV is not found in the calculations but has been observed in gas-phase studies; it is attributed to the formation of a shape resonance. PMID:26896993

  14. Ionic photofragmentation and photoionization of dimethyl ether in the VUV and soft X-ray regions (8.5 80 eV) absolute oscillator strengths for molecular and dissociative photoionization

    NASA Astrophysics Data System (ADS)

    Feng, Renfei; Cooper, Glyn; Brion, C. E.

    2001-08-01

    The branching ratios for molecular and dissociative photoionization of dimethyl ether (CH 3OCH 3, DME) have been measured in the VUV and soft X-ray regions using dipole (e,e+ion) coincidence spectroscopy (˜1 eV FWHM) at equivalent photon energies from the first ionization threshold up to 80 eV. The absolute partial oscillator strengths (cross-sections) for molecular and dissociative photoionization have been determined from recently published absolute photoabsorption oscillator strength data [R. Feng, G. Cooper, C.E. Brion, Chem. Phys. 260 (2000) 391] together with the photoionization branching ratios and the (multi-dissociative-corrected) photoionization efficiency obtained from time-of-flight mass spectra reported in the present work. No stable multiply charged molecular ion(s) from DME have been found in the present work. However, the fact that the photoionization efficiency has been measured as greater than unity above ˜30 eV indicates the existence of multi-dissociative products from Coulomb explosion of multiply charged ions. Appearance potentials of all ion products from DME are also reported. The presently reported results are compared with the previously published data where possible.

  15. Absolute partial and total electron-impact-ionization cross sections for CF4 from threshold up to 500 eV

    NASA Astrophysics Data System (ADS)

    Ma, Ce; Bruce, M. R.; Bonham, R. A.

    1991-09-01

    Electron-impact dissociative ionization of tetrafluoromethane (CF4) was studied with the use of a pulsed electron beam time-of-flight apparatus. The absolute partial ionization cross sections of CF+3, CF+2, CF2+3, CF+, CF2+2, F+, and C+ were measured from threshold up to 500 eV. The total ionization cross section was obtained by charge weighted summing of all the observed partial ionization cross sections. A total cross section for dissociation into neutral fragments was inferred from our total ionization cross section and the total dissociation cross section of Winters and Inokuti [Phys. Rev. A 25, 1420 (1982)]. The present results for the partial ionization cross sections are as much as 9% (CF+3) to 81% (F+) higher than the previously published absolute measurements of Stephan, Deutsch, and Märk [J. Chem. Phys. 83, 5712 (1985)] at 80 eV, but are in agreement with their recently revised estimates for the singly charged ions. We also found that dissociative ionization was a dominant process for electron-impact energies above 30 eV, accounting for 85% of the total dissociation cross section at 80 eV.

  16. Absolute absorption cross sections of ozone at 300 K, 228 K and 195 K in the wavelength region 185-240 nm

    NASA Technical Reports Server (NTRS)

    Yoshino, K.; Parkinson, W. H.; Freeman, D. E.

    1992-01-01

    An account is given of progress of work on absorption cross section measurements of ozone at 300 K, 228 K and 195 K in the wavelength region 185-240 nm. In this wavelength region, the penetration of solar radiation into the Earth's atmosphere is controlled by O2 and O3. The transmitted radiation is available to dissociate trace species such as halocarbons and nitrous oxide. We have recently measured absolute absorption cross sections of O3 in the wavelength region 240-350 nm (Freeman et al., 1985; Yoshino et al., 1988). We apply these proven techniques to the determination of the absorption cross section of O3 at 300 K, 228 K and 195 K throughout the wavelength region 185-240 nm. A paper titled 'Absolute Absorption Cross Section Measurements of Ozone in the Wavelength Region 185-254 nm and the Temperature Dependence' has been submitted for publication in the Journal of Geophysical Research.

  17. Calculations of the Raman photoionization cross section for bound-free transitions in Neon-like Iron

    NASA Astrophysics Data System (ADS)

    Kruse, Michael; Gaffney, James; Iglesias, Carlos; Wilson, Brian

    2016-10-01

    The recent higher-than-expected solar opacity measurements of Bailey et al. on the Sandia Z-machine have raised questions over the accuracy of theoretical opacity models near the solar convection-radiation boundary. Of concern in particular are the Iron opacities for which discrepancies of 30%-400% were found between theory and experiment. Naturally the question has been raised whether theoretical models have neglected to include all the relevant atomic physics processes. In this talk we discuss the effects of the hitherto neglected two-photon ionization cross section for bound-free transitions in Neon-like Iron (a prominent charge state in the solar convection-radiation region). The calculations proceed by solving the Schroedinger equation for an electron moving in a parameterized mean-field potential that has been fitted to experimental data. The required dipole transition strength is calculated by the Dalgarno and Lewis method which exactly recovers the summation over the infinite set of intermediate states between the initial and final state. Conclusions are given with respect to opacity models.

  18. Experimental Studies of Electron Impact Phenomena: (i) Absolute Elastic Differential Cross Section Measurements of Carbon-Monoxide Nitrogen Molecule, and Carbon-Dioxide Using a Refined Relative Flow Technique, (ii) Differential Cross Section Measurements for Excitation of Electronic Levels of Carbon-Monoxide by Electron Impact, (iii) Absolute Total Scattering Cross Section Measurements for Electron Impact on Krypton, Oxygen Molecule, and Carbon-Monoxide

    NASA Astrophysics Data System (ADS)

    Kanik, Isik

    1988-12-01

    Absolute elastic differential scattering cross sections (DCS) for electron impact on CO, N_2 , and CO_2 in the energy range 20-100 eV and angular range 20^circ -120^circ were measured. A crossed beam scattering geometry was employed and the results were obtained using a relative flow technique in which the DCS of CO and CO_2 were compared directly to the DCS of helium at each angle and energy and the DCS of N_2 was compared directly to the DCS of CO. The results of the elastic DCS of neon are also presented as a check on the experimental procedure. Differential cross section measurements for excitation of the electronic features (a^3Pi , a^'^3Sigma ^+, d^3Delta, and A^1Pi) of CO by electron impact have been carried out by JPL group (Peter Zetner and Sandor Trajmar). These data have been analyzed and differential cross sections were obtained for the impact energies 12.5 eV and 15.0 eV by using a computer unfolding program that employes flux corrected Franck-Condon factors and calibration scheme developed jointly with the JPL group. Details of the routine for extracting the DCS are presented. Absolute total scattering cross section measurements were carried out for electron impact on Kr, O_2 , and CO. The results were obtained using a linear attenuation technique in the 5-300 eV incident energy range. The present results have an assigned error of 3% and generally found to be in good agreement with other experimental data.

  19. Measurement of Absolute Excitation Cross Sections in Highly-Charged Ions Using Electron Energy Loss and Merged Beams

    NASA Technical Reports Server (NTRS)

    Chutjian, A.; Smith, Steven J.; Lozano, J.

    2002-01-01

    There is increasing emphasis during this decade on understanding energy balance and phenomena observed in high electron temperature plasmas. The UV spectral return from FUSE, the X-ray spectral return from the HETG on Chandra and the LETGS 011 XMM-Newton are just beginning. Line emissions are almost entirely from highly-charged ions (HCIs) of C, N, 0, Ne, Mg, S, Si, Ca, and Fe. The Constellation-X mission will provide X-ray spectroscopy up to photon energies of 0.12 nm (10 keV) where primary line emitters will be HCIs. A variety of atomic parameters are required to model the stellar and solar plasma. These include cross sections for excitation, ionization, charge-exchange, X-ray emission, direct and indirect recombination, lifetimes and branching ratios, and dependences on l, m mixing by external E and B fields. In almost all cases the atomic quantities are calculated, and few comparisons to experiment have been carried out. Collision strengths and Einstein A-values are required to convert the observed spectral intensities to electron temperatures and densities in the stellar plasma. The JPL electron energy-loss and merged beam approach has been used to measure absolute collision strengths in a number of ions, with critical comparison made to the best available theories.

  20. Electron scattering from hexafluoride molecules: WF6 and C2F6. Absolute total cross section measurements from 1 to 250 eV

    NASA Astrophysics Data System (ADS)

    Szmytkowski, Czeslaw; Mozejko, Pawel; Kasperski, Grzegorz; Ptasinska-Denga, Elzbieta

    2000-01-01

    Electron-scattering absolute total cross sections for tungsten hexafluoride (WF6) and hexafluorethane (C2F6) molecules have been measured in a linear transmission electron-beam experiment within the impact energy range from about 1 to 250 eV. For electron scattering from WF6 the cross section shows a prominent resonant-like peak centred at 3 eV and a very broad enhancement in the energy range between 20 and 70 eV overlaid with some much less pronounced features. The cross section for C2F6 has two resonant structures at 5 and 9 eV, respectively, and a very broad hump ranging from 20 to 60 eV with a distinct shoulder near 20 eV. Comparison of the e--C2F6 total cross section with available low-energy data from other experiments is made. The effect of fluorination is indicated.

  1. Absolute oscillator strengths for the valence and inner (P 2p,2s) shell photoabsorption, photoionization, and ionic photofragmentation of PF 3

    NASA Astrophysics Data System (ADS)

    Au, Jennifer W.; Brion, C. E.

    1997-08-01

    Absolute oscillator strengths (cross-sections) for the photoabsorption of phosphorus pentafluoride (PF 5) have been measured for the first time in the valence and phosphorus 2p discrete regions using high-resolution (0.0-0.1 eV fwhm), dipole ( e, e) spectroscopy. Long-range data (10-300 eV) have also been obtained at lower resolution (1 eV fwhm), from which the absolute oscillator strength scale has been determined using the valence-shell Thomas-Reiche-Kuhn sum-rule. The accuracy of the present measurement has been tested using the S(-2) sum rule normalization. Evaluation of the S(-2) sum using the presently reported absolute photoabsorption oscillator strength data gives a dipole polarizabilit for PF 5 in good agreement with the experimental value. The photoionization efficiencies, photoion branching ratios, and absolute partial oscillator strengths for molecular and dissociative photoionization have also been determined for PF 5 by dipole ( e, e+ion) coincidence spectroscopy from the first ionization threshold up to and above the phosphorus 2p edge.

  2. Absolute cascade-free cross-sections for the 2S to 2P transition in Zn(+) using electron-energy-loss and merged-beams methods

    NASA Technical Reports Server (NTRS)

    Smith, Steven J.; Man, K.-F.; Chutjian, A.; Mawhorter, R. J.; Williams, I. D.

    1991-01-01

    Absolute cascade-free excitation cross-sections in an ion have been measured for the resonance 2S to 2P transition in Zn(+) using electron-energy-loss and merged electron-ion beams methods. Measurements were carried out at electron energies of below threshold to 6 times threshold. Comparisons are made with 2-, 5-, and 15-state close-coupling and distorted-wave theories. There is good agreement between experiment and the 15-state close-coupling cross-sections over the energy range of the calculations.

  3. Absolute cascade-free cross-sections for the 2S to 2P transition in Zn(+) using electron-energy-loss and merged-beams methods

    NASA Technical Reports Server (NTRS)

    Smith, Steven J.; Man, K.-F.; Chutjian, A.; Mawhorter, R. J.; Williams, I. D.

    1991-01-01

    Absolute cascade-free excitation cross-sections in an ion have been measured for the resonance 2S to 2P transition in Zn(+) using electron-energy-loss and merged electron-ion beams methods. Measurements were carried out at electron energies of below threshold to 6 times threshold. Comparisons are made with 2-, 5-, and 15-state close-coupling and distorted-wave theories. There is good agreement between experiment and the 15-state close-coupling cross-sections over the energy range of the calculations.

  4. Absolute and relative surrogate measurements of the uranium-236(n,f) cross section as a probe of angular momentum effects

    NASA Astrophysics Data System (ADS)

    Lyles, Bethany Faye

    The absolute surrogate technique and the Surrogate Ratio Method (SRM) were used to deduce the 236U(n,f) cross section over an equivalent neutron energy range of 0.1 to 20 MeV for the absolute measurement and 0.8 to 20 MeV for the relative measurement. A 42 MeV 3He2+ beam from the 88--Inch Cyclotron at Lawrence Berkeley National Laboratory was used to perform a (3He,alpha) pickup reaction on targets of 235U (Jpi=7/2 --) and 238U (Jpi=0+) and the fission decay probabilities were determined. The 235U( 3He,alphaf) and 238U(3He,alphaf) reactions were surrogates for 233U(n,f) and 236U(n,f), respectively. Using the absolute surrogate technique, the experimentally determined 238U(3He,alpha) fission probability was multiplied by a calculated neutron absorption cross section to obtain the 236 U(n,f) cross section. Using the SRM, a ratio of the experimentally determined fission probabilities, 238U(3He,alphaf) to 235U(3He,alphaf), was extracted and multiplied by the evaluated 233U(n,f) cross section to obtain the 236U(n,f) cross section. Neither the absolute surrogate nor the SRM used in this case explicitly accounted for Jpi-dependence of the fission probabilities. The cross sections extracted using the Surrogate Method were compared to directly measured cross sections and theoretical predictions. The absolute surrogate 236U(n,f) cross section trended well with the evaluated nuclear data below 3.3 MeV, but was beset with target contamination above this energy, whereas the SRM result agreed with the evaluated nuclear data to within 10% at neutron energies from 3.5 to 20 MeV and exhibited significant deviations in the low energy regime. The deduced surrogate 236U(n,f) cross section was determined as a function of the angle of the alpha particle ejectile in the direct reaction to explore different angular momentum population distributions in the compound nucleus and their effects on the extracted fission probabilities. The 236U(n,f) cross sections extracted using both the

  5. A novel setup for the determination of absolute cross sections for low-energy electron induced strand breaks in oligonucleotides - The effect of the radiosensitizer 5-fluorouracil*

    NASA Astrophysics Data System (ADS)

    Rackwitz, Jenny; Ranković, Miloš Lj.; Milosavljević, Aleksandar R.; Bald, Ilko

    2017-02-01

    Low-energy electrons (LEEs) play an important role in DNA radiation damage. Here we present a method to quantify LEE induced strand breakage in well-defined oligonucleotide single strands in terms of absolute cross sections. An LEE irradiation setup covering electron energies <500 eV is constructed and optimized to irradiate DNA origami triangles carrying well-defined oligonucleotide target strands. Measurements are presented for 10.0 and 5.5 eV for different oligonucleotide targets. The determination of absolute strand break cross sections is performed by atomic force microscopy analysis. An accurate fluence determination ensures small margins of error of the determined absolute single strand break cross sections σ SSB . In this way, the influence of sequence modification with the radiosensitive 5-Fluorouracil (5FU) is studied using an absolute and relative data analysis. We demonstrate an increase in the strand break yields of 5FU containing oligonucleotides by a factor of 1.5 to 1.6 compared with non-modified oligonucleotide sequences when irradiated with 10 eV electrons.

  6. Absolute cross sections for binary-encounter electron ejection by 95-MeV/u {sup 36}Ar{sup 18+} penetrating carbon foils

    SciTech Connect

    De Filippo, E.; Lanzano, G.; Aiello, S.; Arena, N.; Geraci, M.; Pagano, A.; Rothard, H.; Volant, C.; Anzalone, A.; Giustolisi, F.

    2003-08-01

    Doubly differential electron velocity spectra induced by 95-MeV/u {sup 36}Ar{sup 18+} from thin carbon foils were measured at GANIL (Caen, France) by means of the ARGOS multidetector and the time-of-flight technique. The spectra allow us to determine absolute singly differential cross sections as a function of the emission angle. Absolute doubly differential cross sections for binary encounter electron ejection from C targets are compared to a transport theory, which is based on the relativistic electron impact approximation for electron production and which accounts for angular deflection, energy loss, and also energy straggling of the transmitted electrons. For the thinnest targets, the measured peak width is in good agreement with experimental data obtained with a different detection technique. The theory underestimates the peak width but provides (within a factor of 2) the correct peak intensity. For the thickest target, even the peak shape is well reproduced by theory.

  7. Absolute doubly differential cross sections for ionization of adenine by 1.0-MeV protons

    SciTech Connect

    Iriki, Y.; Kikuchi, Y.; Imai, M.; Itoh, A.

    2011-09-15

    Double-differential ionization cross sections of adenine (C{sub 5}H{sub 5}N{sub 5}) by 1.0-MeV protons have been measured using a vapor-phase adenine target. Ejected electrons were analyzed by a 45 deg. parallel-plate electrostatic spectrometer in an electron energy range from 1 to 1000 eV at electron emission angles from 15 deg. to 165 deg. The effective target thickness of adenine was determined by a Rutherford forward scattering method and a vapor deposition method. Present data are in good agreement with recent calculations. Comparisons were made with other data on various hydrocarbon molecules. It was found that the ionization cross sections of these molecules can be scaled fairly well in terms of the total number of valence electrons.

  8. Absolute excited-state absorption cross section and fluorescence quantum efficiency of Cr/sup 3 +/: gadolinium scandium gallium garnet

    SciTech Connect

    Seelert, W.; Strauss, E.

    1987-10-01

    Excited-state properties of the laser material Cr/sup 3 +/:Gd/sub 3/Sc/sub 2/(GaO/sub 4/)/sub 3/ were determined by a photocaloric technique. The excited-state absorption cross section at 650 nm is (3.6 +- 0.6)10/sup -20/ cm/sup 2/, and the fluorescence quantum efficiency at ambient temperature is (91 +- 1)%.

  9. Absolute and Relative Surrogate Measurements of the 236U(n,f) Cross Section as a Probe for Angular Momentum Effects

    SciTech Connect

    Lyles, B; Bernstein, L; Burke, J; Escher, J; Thompson, I; Dietrich, F; Phair, L; Bleuel, D; Gibelin, J; Wiedeking, M; McMahan, M; Rodroguez-Vieitez, E; Clark, R; Macchiavelli, A; Lesher, S; Darakchieva, B; Evtimova, M; Beausang, C; Fallon, P

    2007-04-03

    Using both the absolute and relative surrogate techniques, the {sup 236}U(n,f) cross section was deduced over an equivalent neutron energy range of 0 to 20 MeV. A 42 MeV {sup 3}He beam from the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory was used to perform a ({sup 3}He,{alpha}) pickup reaction on targets of {sup 235}U (J{sup {pi}}=7/2{sup -}) and {sup 238}U (J{sup {pi}}=0{sup +}) and the fission decay probabilities were determined. The {sup 235}U({sup 3}He,{alpha}f) and {sup 238}U({sup 3}He,{alpha}f) were surrogates for {sup 233}U(n,f) and {sup 236}U(n,f), respectively. The cross sections extracted using the Surrogate Method were compared to directly measured cross sections. The sensitivity of these cross sections to the J{sup {pi}}-population distributions was explored.

  10. Benchmark experiment for electron-impact ionization of argon: Absolute triple-differential cross sections via three-dimensional electron emission images

    SciTech Connect

    Ren Xueguang; Senftleben, Arne; Pflueger, Thomas; Dorn, Alexander; Ullrich, Joachim; Bartschat, Klaus

    2011-05-15

    Single ionization of argon by 195-eV electron impact is studied in an experiment, where the absolute triple-differential cross sections are presented as three-dimensional electron emission images for a series of kinematic conditions. Thereby a comprehensive set of experimental data for electron-impact ionization of a many-electron system is produced to provide a benchmark for comparison with theoretical predictions. Theoretical models using a hybrid first-order and second-order distorted-wave Born plus R-matrix approach are employed to compare their predictions with the experimental data. While the relative shape of the calculated cross section is generally in reasonable agreement with experiment, the magnitude appears to be the most significant problem with the theoretical treatment for the conditions studied in the present work. This suggests that the most significant challenge in the further development of theory for this process may lie in the reproduction of the absolute scale rather than the angular dependence of the cross section.

  11. Tracing multiple scattering patterns in absolute (e,2e) cross sections for H{sub 2} and He over a 4{pi} solid angle

    SciTech Connect

    Ren, X.; Senftleben, A.; Pflueger, T.; Dorn, A.; Ullrich, J.; Colgan, J.; Pindzola, M. S.; Al-Hagan, O.; Madison, D. H.; Bray, I.; Fursa, D. V.

    2010-09-15

    Absolutely normalized (e,2e) measurements for H{sub 2} and He covering the full solid angle of one ejected electron are presented for 16 eV sum energy of both final state continuum electrons. For both targets rich cross-section structures in addition to the binary and recoil lobes are identified and studied as a function of the fixed electron's emission angle and the energy sharing among both electrons. For H{sub 2} their behavior is consistent with multiple scattering of the projectile as discussed before [Al-Hagan et al., Nature Phys. 5, 59 (2009)]. For He the binary and recoil lobes are significantly larger than for H{sub 2} and partly cover the multiple scattering structures. To highlight these patterns we propose a alternative representation of the triply differential cross section. Nonperturbative calculations are in good agreement with the He results and show discrepancies for H{sub 2} in the recoil peak region. For H{sub 2} a perturbative approach reasonably reproduces the cross-section shape but deviates in absolute magnitude.

  12. Tracing multiple scattering patterns in absolute (e,2e) cross sections for H2 and He over a 4π solid angle

    NASA Astrophysics Data System (ADS)

    Ren, X.; Senftleben, A.; Pflüger, T.; Dorn, A.; Colgan, J.; Pindzola, M. S.; Al-Hagan, O.; Madison, D. H.; Bray, I.; Fursa, D. V.; Ullrich, J.

    2010-09-01

    Absolutely normalized (e,2e) measurements for H2 and He covering the full solid angle of one ejected electron are presented for 16 eV sum energy of both final state continuum electrons. For both targets rich cross-section structures in addition to the binary and recoil lobes are identified and studied as a function of the fixed electron’s emission angle and the energy sharing among both electrons. For H2 their behavior is consistent with multiple scattering of the projectile as discussed before [Al-Hagan , Nature Phys.PLRAAN1745-247310.1038/nphys1135 5, 59 (2009)]. For He the binary and recoil lobes are significantly larger than for H2 and partly cover the multiple scattering structures. To highlight these patterns we propose a alternative representation of the triply differential cross section. Nonperturbative calculations are in good agreement with the He results and show discrepancies for H2 in the recoil peak region. For H2 a perturbative approach reasonably reproduces the cross-section shape but deviates in absolute magnitude.

  13. Absolute fragmentation cross sections in atom-molecule collisions: Scaling laws for non-statistical fragmentation of polycyclic aromatic hydrocarbon molecules

    SciTech Connect

    Chen, T.; Gatchell, M.; Stockett, M. H.; Alexander, J. D.; Schmidt, H. T.; Cederquist, H.; Zettergren, H.; Zhang, Y.; Rousseau, P.; Maclot, S.; Delaunay, R.; Adoui, L.; Domaracka, A.; Huber, B. A.

    2014-06-14

    We present scaling laws for absolute cross sections for non-statistical fragmentation in collisions between Polycyclic Aromatic Hydrocarbons (PAH/PAH{sup +}) and hydrogen or helium atoms with kinetic energies ranging from 50 eV to 10 keV. Further, we calculate the total fragmentation cross sections (including statistical fragmentation) for 110 eV PAH/PAH{sup +} + He collisions, and show that they compare well with experimental results. We demonstrate that non-statistical fragmentation becomes dominant for large PAHs and that it yields highly reactive fragments forming strong covalent bonds with atoms (H and N) and molecules (C{sub 6}H{sub 5}). Thus nonstatistical fragmentation may be an effective initial step in the formation of, e.g., Polycyclic Aromatic Nitrogen Heterocycles (PANHs). This relates to recent discussions on the evolution of PAHNs in space and the reactivities of defect graphene structures.

  14. Absolute cross sections for electron loss, electron capture, and multiple ionization in collisions of C{sup 3+} with noble gases

    SciTech Connect

    Santos, A. C. F.; Sant'Anna, M. M.; Montenegro, E. C.; Sigaud, G. M.; Melo, W. S.

    2010-07-15

    Absolute charge-state-correlated cross sections for projectile electron loss, electron capture, and target multiple ionization in collisions between C{sup 3+} ions and noble gases have been measured for energies between 1.3 and 3.5 MeV. The data have been compared with other similar absolute cross sections existent in the literature for several projectiles. Calculations for the single-loss-multiple-ionization channel have been performed for the screening mode, using both an extended version of the classical-impulse free-collision model and the plane-wave Born approximation (PWBA), and for the antiscreening mode within the PWBA. The energy dependence of the average number of target active electrons which contribute to the antiscreening has been described by means of a simple function, which is ''universal'' for noble gases but, in principle, projectile dependent. A method has been developed to obtain the number of active target electrons for each subshell in the high-velocity regime, which presented physically reasonable results. Analyses of the dependences of the single-capture and transfer-ionization (SC and TI, respectively) processes on the projectile charge states showed that, for He, equally charged bare and dressed projectiles have very similar cross sections; the latter thus acting as structureless point charges. A behavior similar to that in the SC has been observed for the pure single ionization of He by projectiles with different charge states and of the other noble gases by singly charged projectiles. It has been shown that the q{sup 2} dependence of the pure-single and total-ionization cross sections, predicted by first-order models, is only valid for high-collision velocities. For slower collisions, the electron capture process becomes more relevant and competes with the ionization channel, a feature which grows in importance as the projectile charge state increases.

  15. Absolute state-selected and state-to-state total cross sections for the Ar sup + ( sup 2 P sub 3/2,1/2 )+CO reactions

    SciTech Connect

    Flesch, G.D.; Nourbakhsh, S.; Ng, C.Y. . Ames Laboratory Iowa State University, Ames, Iowa . Department of Chemistry)

    1991-09-01

    Absolute spin--orbit state-selected total cross sections for the reactions, Ar{sup +}({sup 2}{ital P}{sub 3/2,1/2})+CO{r arrow}CO{sup +}+Ar (reaction (1)), C{sup +}+O+Ar (reaction (2)), O{sup +}+C+Ar (reaction (3)), and ArC{sup +}+O (reaction (4)), have been measured in the center-of-mass collision energy ({ital E}{sub c.m.}) range of 0.04--123.5 eV. Absolute spin--orbit state transition total cross sections for the Ar{sup +}({sup 2}{ital P}{sub 3/2,1/2})+CO reactions at {ital E}{sub c.m.} have also been obtained. The appearance energies (AE) for C{sup +}({ital E}{sub c.m.}=6.6{plus minus}0.4 eV) and O{sup +}({ital E}{sub c.m.}=8.6{plus minus}0.4 eV) are in agreement with the thermochemical thresholds for reactions (2) and (3), respectively. The observed AE for reaction (4) yields a lower bound of 0.5 eV for the ArC{sup +} bond dissociation energy. The kinetic energy dependence of the absolute cross sections and the retarding potential analysis of the product ions support that ArC{sup +}, C{sup +}, and O{sup +} are formed via a charge transfer predissociation mechanism, similar to that proposed to be responsible for the formation of O{sup +} (N{sup +}) and ArO{sup +} (ArN{sup +}) in the collisions of Ar{sup +}({sup 2}{ital P}{sub 3/2,1/2})+O{sub 2}(N{sub 2}).

  16. Absolute measurement of the differential cross section for the reaction sup 4 He(. gamma. , p ) sup 3 H from 63 to 71 MeV

    SciTech Connect

    Jones, R.T.; Jenkins, D.A. ); Debevec, P.T.; Harty, P.D.; Knott, J.E. )

    1991-05-01

    Results are presented from a {sup 4}He photodisintegration experiment performed with quasimonochromatic photons using a large solid-angle detector. The tagged-bremsstrahlung technique gave a reliable absolute normalization. In addition, an unambiguous separation of the proton-triton channel from other photodisintegration channels was achieved. A total cross section of 218{plus minus}8 {mu}b was measured at a mean energy of 67{plus minus}4 MeV and Legendre coefficients up to {ital a}{sub 5} were extracted from the angular distributions.

  17. Measurement of absolute charge-exchange cross sections for He{sup 2+} collisions with He and H{sub 2}

    SciTech Connect

    Mawhorter, R. J.; Greenwood, J. B.; Chutjian, A.; Simcic, J.; Haley, T.; Mitescu, C. D.

    2011-11-15

    Reported are total, absolute charge-exchange cross sections for collisions of {sup 3}He{sup 2+} ions with He and H{sub 2}. Measurements are reported at fixed energies between 0.33 and 4.67 keV/amu. Both the present results and earlier results of others are analyzed in terms of available experimental small-angle differential cross sections as a function of collision energy, and hence the geometry of the exit aperture of the gas-collision cells used by the various experimental groups. In addition, the effective length of gas-collision cells is studied using fluid dynamic and molecular flow simulations to address the density patterns near the cell entrance and exit apertures. When small acceptance-angle corrections were applied, the results of present and previous measurements for the single electron capture in these systems were brought into good accord in the relevant energy ranges. Taken in their entirety, the present data for {sup 3}He{sup 2+} with He and H{sub 2} lend themselves to new theoretical calculations of the multichannel charge-exchange cross sections.

  18. Chlorine atom spin orbit branching ratios and total absolute reaction cross-sections for the H+DCl→HD+Cl reaction

    NASA Astrophysics Data System (ADS)

    Hanf, Alexander; Läuter, Almuth; Suresh, Dhanya; Volpp, Hans-Robert; Wolfrum, Jürgen

    2001-05-01

    Chlorine atom spin-orbit product branching ratios and total absolute reaction cross-sections have been measured for the H+DCl→HD+Cl gas-phase reaction for collision energies of E col=1.0, 1.4 and 1.7 eV. The measured Cl*( 2P1/2) atom spin-orbit product branching ratios φ Cl*(1.0 eV)=[ Cl*]/[ Cl+ Cl*]=(0.06±0.02) , φ Cl*(1.4 eV)=(0.07±0.01) , and φ Cl*(1.7 eV)=(0.16±0.01) revealed the increasing importance of a non-adiabatic reaction channel H+DCl→HD+Cl * with increasing collision energy. The measured total absolute reaction cross-sections allow for comparison with results from recent quasi-classical trajectory (QCT) calculations [F.J. Aoiz et al. J. Phys. Chem. A 104 (2000) 10452].

  19. A novel double-focusing time-of-flight mass spectrometer for absolute recoil ion cross sections measurements.

    PubMed

    Sigaud, L; de Jesus, V L B; Ferreira, Natalia; Montenegro, E C

    2016-08-01

    In this work, the inclusion of an Einzel-like lens inside the time-of-flight drift tube of a standard mass spectrometer coupled to a gas cell-to study ionization of atoms and molecules by electron impact-is described. Both this lens and a conical collimator are responsible for further focalization of the ions and charged molecular fragments inside the spectrometer, allowing a much better resolution at the time-of-flight spectra, leading to a separation of a single mass-to-charge unit up to 100 a.m.u. The procedure to obtain the overall absolute efficiency of the spectrometer and micro-channel plate detector is also discussed.

  20. A novel double-focusing time-of-flight mass spectrometer for absolute recoil ion cross sections measurements

    SciTech Connect

    Sigaud, L.; Jesus, V. L. B. de; Ferreira, Natalia

    2016-08-15

    In this work, the inclusion of an Einzel-like lens inside the time-of-flight drift tube of a standard mass spectrometer coupled to a gas cell—to study ionization of atoms and molecules by electron impact—is described. Both this lens and a conical collimator are responsible for further focalization of the ions and charged molecular fragments inside the spectrometer, allowing a much better resolution at the time-of-flight spectra, leading to a separation of a single mass-to-charge unit up to 100 a.m.u. The procedure to obtain the overall absolute efficiency of the spectrometer and micro-channel plate detector is also discussed.

  1. Absolute state-selected total cross sections for the ion-molecule reactions O + (4S,2D,2P)+H2(D2)

    NASA Astrophysics Data System (ADS)

    Li, X.; Huang, Y.-L.; Flesch, G. D.; Ng, C. Y.

    1997-01-01

    Absolute total cross sections for the state-selected reactions of O+(4S,2D,2P)+H2 (D2) have been measured in the center-of-mass collision energy (Ec.m.) range of 0.02-12 eV. The cross sections for OH+ (OD+) from O+(2D)+H2 (D2) are slightly higher than those from O+(4S)+H2 (D2), whereas the OH+ (OD+) cross sections from O+ (2P)+H2 (D2) are ≈40% lower than those from O+(4S)+H2 (D2) and O+ (2D)+H2 (D2). At Ec.m.<0.5 eV, the total cross sections for OH+ (OD+) from O+ (4S)+H2 (D2) and O+(2D)+H2 (D2) are in accord with those predicted by the Langevin-Gioumousis-Stevenson model. Significantly higher cross sections are observed for H+ (D+) and H2+ (D2+) from O+(2D)+H2 (D2) and O+(2P)+H2 (D2), as compared to those from O+(4S)+H2 (D2). The exothermic nature of the O+(2D,2P)+H2 (D2) charge transfer collisions accounts for the high cross sections observed for H2+ (D2+). While the H+ (D+) ions observed in the O+(4S)+H2 (D2) reaction are identified with the H+ (D+)+O+H channel, the H+ (D+) ions from the reactions involving O+(2D) and O+(2P) are associated mostly with the H+ (D+)+OH (OD) channel, the formation of which obeys the spin-conservation rule. The comparison of the sum (σT) of cross sections for OH+ (OD+), H2+ (D2+), and H+ (D+) from O+(4S)+H2 (D2) to those from O+(2D)+H2 (D2) and O+(2P)+H2 (D2) shows that the σTs for O+(4S)+H2 (D2), O+(2D)+H2 (D2), and O+(2P)+H2 (D2) at Ec.m.<0.5 eV are comparable. At Ec.m.>0.5 eV, the σTs for O+(2P)+H2 (D2) are greater than those for O+(2D)+H2 (D2), which in turn are greater than those for O+(4S)+H2 (D2). This observation is attributed to the increase in the number of accessible product channels for reactions involving the excited O+(2D) and O+(2P) reactant ions.

  2. Absorption spectrum and absolute absorption cross sections of CH3O2 radicals and CH3I molecules in the wavelength range 7473-7497 cm(-1).

    PubMed

    Faragó, Eszter P; Viskolcz, Bela; Schoemaecker, Coralie; Fittschen, Christa

    2013-12-05

    The absorption spectrum of CH3O2 radicals and CH3I molecules has been measured in the range 7473-7497 cm(-1). CH3O2 radicals have been generated by 248 nm laser photolysis of CH3I in the presence of O2, and the relative absorption has been measured by time-resolved continuous-wave cavity ring-down spectroscopy (cw-CRDS). Calibration of the relative absorption spectrum has been carried out on three distinct wavelengths by carefully measuring CH3O2 decays under different experimental conditions and extracting the initial radical concentration (and with this the absolute absorption cross sections) by using the well-known rate constant for the CH3O2 self-reaction. The following, pressure-independent absorption cross sections were determined: 3.41 × 10(-20), 3.40 × 10(-20), and 2.11 × 10(-20) cm(2) at 7748.18, 7489.16, and 7493.33 cm(-1). These values are 2-3 times higher than previous determinations ( Pushkarsky, M. B.; Zalyubovsky, S. J.; Miller, T. A. J. Chem. Phys. 2000, 112 (24), 10695 - 10698 and Atkinson, D. B.; Spillman, J. L. J. Phys. Chem. A 2002, 106 (38), 8891 - 8902). The absorption spectrum of the stable precursor CH3I has also been determined and three characteristic sharp absorption lines with absorption cross sections up to 2 × 10(-21) cm(2) have been observed in this wavelength range.

  3. Measurement of Absolute Excitation Cross Sections in Highly-Charged Ions Using Electron Energy Loss and Merged Beams

    NASA Astrophysics Data System (ADS)

    Chutjian, A.; Smith, Steven J.; Lozano, J. A.

    2002-11-01

    There is increasing emphasis within this decade on understanding energy balance and new phenomena observed in high electron temperature plasmas. The UV spectral return from FUSE, and the X-ray spectral return from the HETG on Chandra and the LETGS on XMM-Newton are just beginning. The line emissions are almost entirely from highly-charged ions (HCIs) of C, N, O, Ne, Mg, S, Si, Ca, and Fe. In addition, the Constellation-X mission, currently in the planning stages, will provide high-throughput X-ray spectroscopy up to photon energies of 0.12 nm (10 keV), where the primary line emitters will again be the HCIs. This array of space instruments is providing an overwhelming return of HCI spectral data from a variety of astrophysical objects. Collision strengths and Einstein A-values are required to convert the observed spectral intensities to electron temperatures and densities in the stellar plasma [1]. The JPL electron energy-loss and merged-beams approach [2] has been used to measure absolute collision strengths in a number of ions, with critical comparisons to the best available theories. Experimental methods will be reviewed, and results presented on experimental comparisons to R-Matrix and Breit-Pauli theoretical results in C3+[3], O2+[4], O5+[5], S2+[6], and Fe9+ [7]. Work is planned for comparisons in Mgq+, and higher charge states Fe(10-15)+. J. Lozano thanks the National Research Council for a fellowship though the NASA- NRC program. This work was carried out at the Jet Propulsion Laboratory, California Institute of Technology, and was supported under contract with the National Aeronautics and Space Administration.

  4. Absolute cross sections for near-threshold electron-impact excitation of the 2s 2S-->2p 2P transition in C3+

    NASA Astrophysics Data System (ADS)

    Bannister, M. E.; Chung, Y.-S.; Djurić, N.; Wallbank, B.; Woitke, O.; Zhou, S.; Dunn, G. H.; Smith, A. C.

    1998-01-01

    Absolute total cross sections for electron-impact excitation of the 2s 2S-->2p 2P transition in C3+ were measured from 7.35 eV to 8.45 eV using the merged electron-ion-beams energy-loss technique. The results settle the discrepancy between two previous experiments using the crossed-beams fluorescence method, being in very good agreement with the older results [P. O. Taylor, D. Gregory, G. H. Dunn, R. A. Phaneuf, and D. H. Crandall, Phys. Rev. Lett. 39, 1256 (1977)] but less so with the more recent ones [D. W. Savin, L. D. Gardner, D. B. Reisenfeld, A. R. Young, and J. L. Kohl, Phys. Rev. A 51, 2162 (1995)]. The present measurements are also in good agreement with unitarized Coulomb-Born and close-coupling calculations.

  5. Absolute cross section measurements of neutron-induced fission of 242Pu from 1 to 2.5 MeV

    NASA Astrophysics Data System (ADS)

    Matei, C.; Belloni, F.; Heyse, J.; Plompen, A. J. M.; Thomas, D. J.

    2017-02-01

    The absolute neutron-induced fission cross section of 242Pu was measured at five energies between 1 and 2.5 MeV at the low-scatter neutron measurement facility of the National Physical Laboratory, UK. The measurements are part of an effort to reduce uncertainties of nuclear data related to fast spectrum reactors. The neutron-induced fission results are in good agreement with the Evaluated Nuclear Data File/B-VII.1 but disagree with several recent measurements near the resonance-like structure around 1.1 MeV. Within the same experimental campaign, the spontaneous fission half-life of 242Pu was measured and it is in good agreement with previous results.

  6. Measurement of absolute hadronic branching fractions of D mesons and e+e- -->DD cross sections at Ec.m.=3773 MeV.

    PubMed

    He, Q; Muramatsu, H; Park, C S; Park, W; Thorndike, E H; Coan, T E; Gao, Y S; Liu, F; Artuso, M; Boulahouache, C; Blusk, S; Butt, J; Dambasuren, E; Dorjkhaidav, O; Li, J; Menaa, N; Mountain, R; Nandakumar, R; Randrianarivony, K; Redjimi, R; Sia, R; Skwarnicki, T; Stone, S; Wang, J C; Zhang, K; Csorna, S E; Bonvicini, G; Cinabro, D; Dubrovin, M; Briere, R A; Chen, G P; Chen, J; Ferguson, T; Tatishvili, G; Vogel, H; Watkins, M E; Rosner, J L; Adam, N E; Alexander, J P; Berkelman, K; Cassel, D G; Crede, V; Duboscq, J E; Ecklund, K M; Ehrlich, R; Fields, L; Gibbons, L; Gittelman, B; Gray, R; Gray, S W; Hartill, D L; Heltsley, B K; Hertz, D; Hsu, L; Jones, C D; Kandaswamy, J; Kreinick, D L; Kuznetsov, V E; Mahlke-Krüger, H; Meyer, T O; Onyisi, P U E; Patterson, J R; Peterson, D; Phillips, E A; Pivarski, J; Riley, D; Ryd, A; Sadoff, A J; Schwarthoff, H; Shi, X; Shepherd, M R; Stroiney, S; Sun, W M; Urner, D; Weaver, K M; Wilksen, T; Weinberger, M; Athar, S B; Avery, P; Breva-Newell, L; Patel, R; Potlia, V; Stoeck, H; Yelton, J; Rubin, P; Cawlfield, C; Eisenstein, B I; Gollin, G D; Karliner, I; Kim, D; Lowrey, N; Naik, P; Sedlack, C; Selen, M; Williams, J; Wiss, J; Edwards, K W; Besson, D; Pedlar, T K; Cronin-Hennessy, D; Gao, K Y; Gong, D T; Hietala, J; Kubota, Y; Klein, T; Lang, B W; Li, S Z; Poling, R; Scott, A W; Smith, A; Dobbs, S; Metreveli, Z; Seth, K K; Tomaradze, A; Zweber, P; Ernst, J; Mahmood, A H; Severini, H; Asner, D M; Dytman, S A; Love, W; Mehrabyan, S; Mueller, J A; Savinov, V; Li, Z; Lopez, A; Mendez, H; Ramirez, J; Huang, G S; Miller, D H; Pavlunin, V; Sanghi, B; Shipsey, I P J; Adams, G S; Chasse, M; Cravey, M; Cummings, J P; Danko, I; Napolitano, J

    2005-09-16

    Using 55.8 pb(-1) of e+e- collisions recorded at the psi(3770) resonance with the CLEO-c detector at CESR, we determine absolute hadronic branching fractions of charged and neutral D mesons using a double tag technique. Among measurements for three D0 and six D+ modes, we obtain reference branching fractions B(D0-->K-pi+)=(3.91+/-0.08+/-0.09)% and B(D+-->K-pi+pi+)=(9.5+/-0.2+/-0.3)%, where the uncertainties are statistical and systematic, respectively. Final state radiation is included in these branching fractions by allowing for additional, unobserved, photons in the final state. Using a determination of the integrated luminosity, we also extract the cross sections sigma(e+e- -->D0D0)=(3.60+/-0.07(+0.07)(-0.05)) nb and sigma(e+e- -->D+D-)=(2.79+/-0.07(+0.10)(-0.04)) nb.

  7. A study of the valence shell absolute photoabsorption, photoionisation and photodissociation cross sections and the photoionisation quantum efficiency of carbonyl sulphide

    NASA Astrophysics Data System (ADS)

    Holland, D. M. P.; Shaw, D. A.

    2016-11-01

    The absolute photoabsorption, photoionisation and photodissociation cross sections and the photoionisation quantum efficiency of carbonyl sulphide have been measured using a double ion chamber and synchrotron radiation in the energy range from the ionisation threshold to 24 eV. In addition to the absorption bands associated with well established Rydberg series, some previously unassigned features have been tentatively attributed to an f-type Rydberg series converging onto the B ˜ 2Σ+ state ionisation threshold. Structure appearing in the photodissociation spectrum has been correlated with that observed in earlier fluorescence yields for emission, due mainly to the CS photofragment, occurring between 160 and 300 nm. The photoionisation quantum efficiency reaches a plateau value close to unity for energies above ∼16 eV. The predissociation of Rydberg states into neutral fragments does not appear to affect the photoionisation quantum efficiency of carbonyl sulphide to the extent that is commonly observed in other small molecules. A sum rule analysis has been carried out by combining the present absolute photoabsorption measurements with similar data covering the remaining energy regions.

  8. High resolution absolute absorption cross sections of the B ̃(1)A'-X ̃(1)A' transition of the CH2OO biradical.

    PubMed

    Foreman, Elizabeth S; Kapnas, Kara M; Jou, YiTien; Kalinowski, Jarosław; Feng, David; Gerber, R Benny; Murray, Craig

    2015-12-28

    Carbonyl oxides, or Criegee intermediates, are formed from the gas phase ozonolysis of alkenes and play a pivotal role in night-time and urban area atmospheric chemistry. Significant discrepancies exist among measurements of the strong B ̃(1)A'-X ̃(1)A' electronic transition of the simplest Criegee intermediate, CH2OO in the visible/near-UV. We report room temperature spectra of the B ̃(1)A'-X ̃(1)A' electronic absorption band of CH2OO acquired at higher resolution using both single-pass broadband absorption and cavity ring-down spectroscopy. The new absorption spectra confirm the vibrational structure on the red edge of the band that is absent from ionization depletion measurements. The absolute absorption cross sections over the 362-470 nm range are in good agreement with those reported by Ting et al. Broadband absorption spectra recorded over the temperature range of 276-357 K were identical within their mutual uncertainties, confirming that the vibrational structure is not due to hot bands.

  9. Assessment of experimental d-PIGE γ-ray production cross sections for 12C, 14N and 16O and comparison with absolute thick target yields

    NASA Astrophysics Data System (ADS)

    Csedreki, L.; Halász, Z.; Kiss, Á. Z.

    2016-08-01

    Measured differential cross sections for deuteron induced γ-ray emission from the reactions 12C(d,pγ)13C, (Eγ = 3089 keV), 14N(d,pγ)15N (Eγ = 8310 keV) and 16O(d,pγ)17O (Eγ = 871 keV) available in the literature were assessed. In order to cross check the assessed γ-ray production cross section data, thick target γ-yields calculated from the differential cross sections were compared with available measured thick target yields. Recommended differential cross section data for each reaction were deduced for particle induced γ-ray emission (PIGE) applications.

  10. Angular Correlation Between Kx-Rays and Gamma - in a Spherically-Deformed Nuclei and Measurement of Absolute Pair Production Cross-Sections Near Threshold Energies.

    NASA Astrophysics Data System (ADS)

    Khalil, Ali El Sayed

    1982-03-01

    (i) Measurements of the directional correlations between Kx-rays following internal conversion and (gamma) -rays in ('181)Ta have been made the correlation coefficients are:. A(,22)(K(alpha)(,1) - 133(gamma)) = 0.037 (+OR -) 0.012. A(,44)(K(alpha)(,1) - 133(gamma)) = 0.022 (+OR -) 0.017. A(,22)(K(alpha)(,2) - 133(gamma)) = 0.038 (+OR -) 0.017. A(,44)(K(alpha)(,2) - 133(gamma)) = 0.037 (+OR -) 0.029. The anisotropic correlation measurements in ('181)Ta establish the second known case of this phenomenon. The x-rays follow four internally converted transitions from which 38% of the Kx-rays follow electric-quadrupole internal conversion processes. This anisotropy is caused by the perturbation of the wave functions of the atomic electrons by the static nuclear quadrupole moment which causes a mixture of the two-coupled, two-electron states (VBAR)d'(,3/2), 1s(,1/2), J = 2 > and (VBAR)d'(,5/2), 1s(,1/2), J = 2 > with the unperturbed state (VBAR)1s(,1/2), 1s(,1/2), J = 0 >. The K-shell electrons are then in a quantum state which is an admixture of the three states mentioned above, and K-shell internal conversion results in a d'(,3/2) or d'(,5/2) vacancy in the mixed K-shell state. Accordingly, x-rays form the transition between either 2p(,3/2) or the 2p(,1/2) level, to a d'(,3/2) or d'(,5/2) vacancy, following internal conversion, can result in anisotropic x-ray angular distributions relative to the nuclear symmetry axis. This in turn results in anisotropic directional correlations between Kx-rays and nuclear (gamma)-rays. (ii) Absolute electron-positron pair production cross-sections near threshold energies have been screened. A new technique which is called internal source method is developed. Direct measurements of the cross-section using 2.615 Mev, a mixture of (1.33 + 1.77) Mev, and 1.12 Mev on target materials of Z = 26, 29, 50, 82 and 92 have been obtained. The experimental results agree well with the exact screening calculations for low Z materials; systematic

  11. Measurement of the partial photoionization cross sections and asymmetry parameters of S atoms in the photon energy range 10.0-30.0 eV using constant-ionic-state spectroscopy

    SciTech Connect

    Innocenti, Fabrizio; Zuin, Lucia; Costa, Maria L.; Dias, Antonio A.; Morris, Alan; Stranges, Stefano; Dyke, John M.

    2007-04-21

    The partial photoionization cross sections and asymmetry parameters of S atoms have been measured using constant-ionic-state (CIS) spectroscopy in the photon energy range 10.0-30.0 eV. The ionizations investigated in these CIS experiments are the (3p){sup -1} ionizations S{sup +}({sup 4}S)(leftarrow)S({sup 3}P), S{sup +}({sup 2}D)(leftarrow)S({sup 3}P), and S{sup +}({sup 2}P)(leftarrow)S({sup 3}P). For the first time Rydberg series which converge to the fourth ionization limit have been observed and assignments of these series have been proposed. These correspond to excitations to Rydberg states that are parts of series which converge to the fourth ionization limit, S{sup +}({sup 4}P)(leftarrow)S({sup 3}P) (3s){sup -1}, and autoionize to the lower S{sup +}({sup 4}S), S{sup +}({sup 2}D), or S{sup +}({sup 2}P) states. For each series observed in the CIS spectra photoelectron angular distribution studies, combined with other evidence, has allowed the angular momentum character of the free electron on autoionization to be determined.

  12. Absolute cross sections for excitation of the 2s 2S-->2p 2P transition in B2+ and for electron-impact single ionization of B2+

    NASA Astrophysics Data System (ADS)

    Woitke, O.; Djurić, N.; Dunn, G. H.; Bannister, M. E.; Smith, A. C.; Wallbank, B.; Badnell, N. R.; Pindzola, M. S.

    1998-12-01

    Absolute cross sections for electron-impact excitation of the 2s 2S-->2p 2P transition of B2+ measured between 5.4 and 7.0 eV are presented. The results are in good agreement with the R-matrix-with-pseudostates (RMPS) calculation of Marchalant et al. [J. Phys. B 30, L435 (1997)]. Also presented are cross sections for electron-impact single ionization of B2+, including measurements between 25 and 200 eV and calculations using the RMPS and time-dependent close-coupling methods. The measured ionization cross sections are about 14% higher near the peak than previous measurements by Crandall et al. [Phys. Rev. A 34, 1757 (1986)], but agree well with experimental data of Hofmann et al. [Z. Phys. D 16, 113 (1990)] and with the present and other theoretical predictions.

  13. Absolute Integral Cross Sections for the State-selected Ion-Molecule Reaction N2+(X2Σg+ v+ = 0-2) + C2H2 in the Collision Energy Range of 0.03-10.00 eV

    NASA Astrophysics Data System (ADS)

    Xu, Yuntao; Xiong, Bo; Chung Chang, Yih; Ng, C. Y.

    2016-08-01

    Using the vacuum ultraviolet laser pulsed field ionization-photoion source, together with the double-quadrupole-double-octopole mass spectrometer developed in our laboratory, we have investigated the state-selected ion-molecule reaction {{{{N}}}2}+({X}2{{{{Σ }}}{{g}}}+; v + = 0-2, N+ = 0-9) + C2H2, achieving high internal-state selectivity and high kinetic energy resolution for reactant {{{{N}}}2}+ ions. The charge transfer (CT) and hydrogen-atom transfer (HT) channels, which lead to the respective formation of product {{{C}}}2{{{{H}}}2}+ and N2H+ ions, are observed. The vibrationally selected absolute integral cross sections for the CT [σ CT(v +)] and HT [[σ HT(v +)] channels obtained in the center-of-mass collision energy (E cm) range of 0.03-10.00 eV reveal opposite E cm dependences. The σ CT(v +) is found to increase as E cm is decreased, and is consistent with the long-range exothermic CT mechanism, whereas the E cm enhancement observed for the σ HT(v +) suggests effective coupling of kinetic energy to internal energy, enhancing the formation of N2H+. The σ HT(v +) curve exhibits a step at E cm = 0.70-1.00 eV, suggesting the involvement of the excited {{{C}}}2{{{{H}}}2}+({A}2{{{{Σ }}}{{g}}}+) state in the HT reaction. Contrary to the strong E cm dependences for σ CT(v +) and σ HT(v +), the effect of vibrational excitation of {{{{N}}}2}+ on both the CT and HT channels is marginal. The branching ratios and cross sections for the CT and HT channels determined in the present study are useful for modeling the atmospheric compositions of Saturn's largest moon, Titan. These cross sections and branching ratios are also valuable for benchmarking theoretical calculations on chemical dynamics of the titled reaction.

  14. Accurate absolute measurements of the Raman backscattering differential cross-section of water and ice and its dependence on the temperature and excitation wavelength

    NASA Astrophysics Data System (ADS)

    Plakhotnik, Taras; Reichardt, Jens

    2017-06-01

    Measurements of Raman backscattering spectra between -15 °C and 22 °C in liquid water (including its supercooled state) and in polycrystalline ice (-35 °C to 0 °C) at two excitation wavelengths (407 and 532 nm) are presented. It is found that the spectrum-integrated backscattering cross-section of the 3400 cm-1 band is about 1.2 times larger for ice in comparison to liquid water. The excitation-wavelength dependence of the cross-section in ice is very close to that in water. A discontinuous change of the spectrum is observed upon phase transition at 0 °C. The results are applicable to preliminary calibration of lidar systems designed for water content surveys in the atmosphere.

  15. Absolute and relative cross section measurements of 237Np(n,f) and 238U(n,f) at the National Physical Laboratory

    NASA Astrophysics Data System (ADS)

    Salvador-Castiñeira, Paula; Hambsch, Franz-Josef; Göök, Alf; Vidali, Marzio; Hawkes, Nigel P.; Roberts, Neil J.; Taylor, Graeme C.; Thomas, David J.

    2017-09-01

    Cross section measurements in the fast energy region are being demanded as one of the key ingredients for modelling Generation-IV nuclear power plants. However, in facilities where there are no time-of-flight possibilities or it is not convenient to use them, using the 235U(n,f) cross section as a benchmark would require a careful knowledge of the room scatter in the experimental area. In this paper we present measurements of two threshold reactions, 238U(n,f) and 237Np(n,f), that could become a standard between their fission threshold and 2.5 MeV, if the discrepancies shown in the evaluations and in some experimental data can be solved. The preliminary results are in agreement with the present ENDF/B-VII.1 evaluation.

  16. Chemiluminescence from the Ca*(/sup 3/P) + SF/sub 6/ reaction: absolute cross section, photon yields, and electronic branching

    SciTech Connect

    Verdasco, E.; Rabanos, V.S.; Aoiz, F.J.; Urena, A.G.

    1987-04-09

    A study of the chemiluminescence under single-collision conditions of the reaction of the metastable Ca(4s4p /sup 3/P/sup 0/) of atomic calcium with SF/sup 6/ is presented. Chemiluminescence cross sections and photon yields for production of various CaF (A,B) band systems are also reported. The observed electronic branching ratio sigma/sub A//sigma/sub B/ is 4.77, and a comparison with several statistical model calculations is also discussed.

  17. Measurement of absolute cross sections for excitation of the 2s(2) S-1 -> 2s2p P-1 degrees transition in O+4

    NASA Technical Reports Server (NTRS)

    Smith, S. J.; Djuric, N.; Lozano, J. A.; Berrington, K. A.; Chutjian, A.

    2005-01-01

    Experimental cross sections are reported for the 1s(2)2s(2) S-1 -> 1s(2)2s2p P-1(o) transition in O+4 located at 19.689 eV. Use is made of the electron energy-loss method, using a merged electron-ion beam geometry. The center-of-mass interaction energies for the measurements in the S-1 -> P-1(o) transition are in the range 18 eV ( below the threshold) to 30 eV. Data are compared with other previous electron energy-loss measurements and with results of a 26 term R-matrix calculation that includes fine structure explicitly via the Breit-Pauli Hamiltonian. Clear resonance enhancement is observed in all experimental and theoretical results near the threshold for this S-1 -> P-1(o) transition.

  18. Absolute Differential Cross-Sections for Elastic PION(+/-)/PROTON Scattering at 30 Less than or Equal to T(pion) Less than or Equal to 140 Mev

    NASA Astrophysics Data System (ADS)

    Brack, Jeffrey Thomas

    Differential cross sections for elastic pi^{+/-}p scattering have been measured at TRIUMF for 10 incident pion energies in three separate experiments at 66.8 <= T_{pi} <= 138.8 MeV, Tpi = 66.8 MeV (pi^+p only), and 30 <= T_{pi} <= 66.8 MeV, using three independent techniques. Typical statistical accuracies are 1-3% and normalization uncertainties are 1.2-3.0%. Extensive experimental checks were employed to minimize systematic errors. Incident pion beam rates were varied by a factor of 5, target thickness was varied by a factor of 10, different target compositions were used (CH_2 and CH_{1.1 }), and derangements of the detector geometry tested the reproducibility of the cross sections under widely varying conditions. Three separate Monte Carlo routines were used. All measurements used solid targets. Thin scintillators and time-of-flight (TOF) techniques were used to count and identify particles incident on the targets and to detect the scattered pions. Recoil protons were detected in coincidence with the scattered pions in two of the three experiments. At the upper range of incident pion energies (66.8 to 138 MeV), a two-arm coincidence technique was used in which proton detection was similar to pion detection (TOF). At the three lowest incident pion energies, an active target technique was used in which the recoil particles were detected by means of the light generated within the CH_ {1.1} scintillator-target. These are the only elastic pip coincidence measurements by any experimental group below 140 MeV incident pion energy. At 66.8 MeV, a third technique was used in which no recoil particles were detected. At incident pion energies of 100 MeV and above, all pi^{+/-}p results from these three measurements are in good agreement with previous measurements, as are the pi ^-p results at all energies. However, while the pi^{+/-}p results of these three experiments are consistent within experimental error at the overlapping energy of 66.8 MeV, they are 10-25% lower than

  19. Measurement of Absolute Cross Sections for Excitation of the 2s^2 ^1S - 2s2p ^1P^o Transition in O^4+

    NASA Astrophysics Data System (ADS)

    Smith, Steven J.; Berrington, K. A.

    2005-05-01

    Experimental electron excitation cross sections are reported for the 2s^2 1S - 2s2p^ 1P^o transitions in O^4+ located at 19.689 eV. The JPL electron-cyclotron resonance ion source is utilized [1], along with the electron energy loss method, in a merged electron-ion beams geometry[2]. The center-of-mass interaction energies for the measurements are in the range 18 eV (below threshold) to 30 eV. Data are compared with results of a 26-term R-matrix calculation that includes fine structure explicitly via the Breit-Pauli Hamiltonian [3]. There is good agreement with theoretical results and with previous electron energy-loss measurements [3]. Clear resonance enhancement is observed in both experiment and theoretical results near threshold for this ^1S - ^1P^o transition. J. Lozano and N. Djuric acknowledge support through the NASA-NRC program. This work was carried out at JPL/Caltech and was supported by NASA. [1] J. B. Greenwood, S. J. Smith, A.Chutjian, and E. Pollack, Phys. Rev. A 59 1348, (1999). [2] A. Chutjian, Physica Scripta T110, 203 (2004). [3] M. Bannister et al., Int.J. Mass Spectrometry 192, 39 (1999).

  20. Jet inclusive cross sections

    SciTech Connect

    Del Duca, V.

    1992-11-01

    Minijet production in jet inclusive cross sections at hadron colliders, with large rapidity intervals between the tagged jets, is evaluated by using the BFKL pomeron. We describe the jet inclusive cross section for an arbitrary number of tagged jets, and show that it behaves like a system of coupled pomerons.

  1. Photoionization of Ar VIII

    NASA Astrophysics Data System (ADS)

    Liang, Liang; Jiang, Wen-xian; Zhou, Chao

    2017-01-01

    The photoionization cross section, energy levels and widths of 22 Rydberg series (in the autoionization region) for Na-like Ar VIII were investigated by using of R-matrix method. The relativistic distorted-wave method is used to calculate the radial functions, and QB method of Quigly-Berrington [Quigley et al. 1998] is employed to calculate the resonance levels and widths. We have identified the formant in the figure of the photoionization cross section.

  2. Photoionization of molecular clusters

    NASA Astrophysics Data System (ADS)

    Andres, R. P.; Calo, J. M.

    1981-12-01

    An experimental apparatus consisting of a novel multiple expansion cluster source coupled with a molecular beam system and photoionization mass spectrometer has been designed and constructed. This apparatus has been thoroughly tested and preliminary measurements of the growth kinetics of water clusters and the photoionization cross section of the water dimer have been carried out.

  3. Neutron cross sections

    SciTech Connect

    Not Available

    1988-01-01

    This handbook displays curves of neutron cross sections in the energy range of 0.01 eV to 200 MeV (and associated information) as a function of incident neutron energy. Tables include reference to all data. Information on isomeric state production is also included. This book represents the fourth edition of what was previously known as BNL-325, Neutron Cross Sections, Volume 2, the third edition of which was published in 1976.

  4. Double Photoionization Near Threshold

    NASA Technical Reports Server (NTRS)

    Wehlitz, Ralf

    2007-01-01

    The threshold region of the double-photoionization cross section is of particular interest because both ejected electrons move slowly in the Coulomb field of the residual ion. Near threshold both electrons have time to interact with each other and with the residual ion. Also, different theoretical models compete to describe the double-photoionization cross section in the threshold region. We have investigated that cross section for lithium and beryllium and have analyzed our data with respect to the latest results in the Coulomb-dipole theory. We find that our data support the idea of a Coulomb-dipole interaction.

  5. Absolute cross section for loss of supercoiled topology induced by 10 eV electrons in highly uniform /DNA/1,3-diaminopropane films deposited on highly ordered pyrolitic graphite

    PubMed Central

    Boulanouar, Omar; Fromm, Michel; Bass, Andrew D.; Cloutier, Pierre; Sanche, Léon

    2013-01-01

    It was recently shown that the affinity of doubly charged, 1–3 diaminopropane (Dap2+) for DNA permits the growth on highly ordered pyrolitic graphite (HOPG) substrates, of plasmid DNA films, of known uniform thickness [O. Boulanouar, A. Khatyr, G. Herlem, F. Palmino, L. Sanche, and M. Fromm, J. Phys. Chem. C 115, 21291–21298 (2011)]. Post-irradiation analysis by electrophoresis of such targets confirms that electron impact at 10 eV produces a maximum in the yield of single strand breaks that can be associated with the formation of a DNA− transient anion. Using a well-adapted deterministic survival model for the variation of electron damage with fluence and film thickness, we have determined an absolute cross section for strand-break damage by 10 eV electrons and inelastic scattering attenuation length in DNA-Dap complex films. PMID:23927289

  6. Absolute cross section for loss of supercoiled topology induced by 10 eV electrons in highly uniform /DNA/1,3-diaminopropane films deposited on highly ordered pyrolitic graphite

    SciTech Connect

    Boulanouar, Omar; Fromm, Michel; Bass, Andrew D.; Cloutier, Pierre; Sanche, Léon

    2013-08-07

    It was recently shown that the affinity of doubly charged, 1-3 diaminopropane (Dap{sup 2+}) for DNA permits the growth on highly ordered pyrolitic graphite (HOPG) substrates, of plasmid DNA films, of known uniform thickness [O. Boulanouar, A. Khatyr, G. Herlem, F. Palmino, L. Sanche, and M. Fromm, J. Phys. Chem. C 115, 21291–21298 (2011)]. Post-irradiation analysis by electrophoresis of such targets confirms that electron impact at 10 eV produces a maximum in the yield of single strand breaks that can be associated with the formation of a DNA{sup −} transient anion. Using a well-adapted deterministic survival model for the variation of electron damage with fluence and film thickness, we have determined an absolute cross section for strand-break damage by 10 eV electrons and inelastic scattering attenuation length in DNA-Dap complex films.

  7. Absolute cross section for loss of supercoiled topology induced by 10 eV electrons in highly uniform /DNA/1,3-diaminopropane films deposited on highly ordered pyrolitic graphite

    NASA Astrophysics Data System (ADS)

    Boulanouar, Omar; Fromm, Michel; Bass, Andrew D.; Cloutier, Pierre; Sanche, Léon

    2013-08-01

    It was recently shown that the affinity of doubly charged, 1-3 diaminopropane (Dap2+) for DNA permits the growth on highly ordered pyrolitic graphite (HOPG) substrates, of plasmid DNA films, of known uniform thickness [O. Boulanouar, A. Khatyr, G. Herlem, F. Palmino, L. Sanche, and M. Fromm, J. Phys. Chem. C 115, 21291-21298 (2011)]. Post-irradiation analysis by electrophoresis of such targets confirms that electron impact at 10 eV produces a maximum in the yield of single strand breaks that can be associated with the formation of a DNA- transient anion. Using a well-adapted deterministic survival model for the variation of electron damage with fluence and film thickness, we have determined an absolute cross section for strand-break damage by 10 eV electrons and inelastic scattering attenuation length in DNA-Dap complex films.

  8. Pediatric obesity and depression: a cross-sectional analysis of absolute BMI as it relates to children's depression index scores in obese 7- to 17-year-old children.

    PubMed

    Benson, Levi P; Williams, Ronald J; Novick, Marsha B

    2013-01-01

    Depression and obesity are important in children because they affect health in childhood and later life. The exact relationship between obesity and depression, especially in children, remains undefined. Using a cross-sectional chart review design, our study looked at a weight management clinic-based sample of 117 obese children, 7 to 17 years old, to determine the relationship between absolute BMI and depression as measured by the Children's Depression Index (CDI) while accounting for confounders, such as the child's medical problems, physical activity, and family structure. There was no correlation between depression as measured by the CDI and increasing BMI in obese children seeking weight management. However, we did demonstrate a positive correlation between depression and paternal absence and daily television/computer/video game time. Clinicians should encourage decreasing screen time and might consider family therapy for obese children in families that lack paternal involvement.

  9. Absolute cross section for loss of supercoiled topology induced by 10 eV electrons in highly uniform /DNA/1,3-diaminopropane films deposited on highly ordered pyrolitic graphite.

    PubMed

    Boulanouar, Omar; Fromm, Michel; Bass, Andrew D; Cloutier, Pierre; Sanche, Léon

    2013-08-07

    It was recently shown that the affinity of doubly charged, 1-3 diaminopropane (Dap(2+)) for DNA permits the growth on highly ordered pyrolitic graphite (HOPG) substrates, of plasmid DNA films, of known uniform thickness [O. Boulanouar, A. Khatyr, G. Herlem, F. Palmino, L. Sanche, and M. Fromm, J. Phys. Chem. C 115, 21291-21298 (2011)]. Post-irradiation analysis by electrophoresis of such targets confirms that electron impact at 10 eV produces a maximum in the yield of single strand breaks that can be associated with the formation of a DNA(-) transient anion. Using a well-adapted deterministic survival model for the variation of electron damage with fluence and film thickness, we have determined an absolute cross section for strand-break damage by 10 eV electrons and inelastic scattering attenuation length in DNA-Dap complex films.

  10. Theoretical treatment of double photoionization of helium using a B-spline implementation of exterior complex scaling

    SciTech Connect

    McCurdy, C. William; Horner, Daniel A.; Rescigno, Thomas N.; Martin, Fernando

    2004-02-19

    Calculations of absolute triple differential and single differential cross sections for helium double photoionization are performed using an implementation of exterior complex scaling in B-splines. Results for cross sections, well-converged in partial waves, are presented and compared with both experiment and earlier theoretical calculations. These calculations establish the practicality and effectiveness of the complex B-spline approach to calculations of double ionization of atomic and molecular systems.

  11. Photo-ionization rate coefficients for the rare gases

    NASA Astrophysics Data System (ADS)

    Pang, Xuexia

    2005-01-01

    By introducing the converting method from electron-impact ionization cross sections to rate coefficients through using a semi-experiential formula, we try to probe a semi-experiential formula for converting the photo-ionization cross sections into photo-ionization rate coefficient. It"s found that photo-ionization rate coefficient is direct proportion to photo-ionization cross sections, the rate S is related with light resource.

  12. Absolute Charge Exchange Cross Sections for C^3,4,5,6+, N^4,5+, O^5,6,7+ , and Ne^7,8+ Collisions with H2O, CH4, CO, and CO2

    NASA Astrophysics Data System (ADS)

    Mawhorter, Richard; Djuric, Nada; Hossain, Sabbir; Macaskill, John; Smith, Steven J.; Chutjian, Ara

    2006-05-01

    The success of the Deep Impact and Stardust missions is advancing our understanding of the structure and composition of comets. This information drives and enhances ongoing cometary EUV and X-ray studies. In turn, our experimental absolute charge exchange cross sections for collisions of highly-charged solar wind ions with cometary gases are necessary for detailed modeling and analysis of these studies. For systems studied earlier, these data agree with the previous measurements made with smaller apertures [1], demonstrating reproducibility and complete angular collection. The ion beam accelerating potential was typically 7 kV, which yields ion velocities consistent with the fast component of the solar wind. Slow solar wind velocity data for O^6+ on CO and CO2 will also be presented. This work was carried out at JPL/Caltech, and was supported through contract with NASA. N. Djuric and S. Hossain also acknowledge support through the NASA-NRC program. [1] J.B. Greenwood, et al., Phys. Rev A 63, 062707 (2001).

  13. Concurrent Application of ANC and THM to assess the 13C(α, n)16O Absolute Cross Section at Astrophysical Energies and Possible Consequences for Neutron Production in Low-mass AGB Stars

    NASA Astrophysics Data System (ADS)

    Trippella, O.; La Cognata, M.

    2017-03-01

    The {}13{{C}}{(α ,n)}16{{O}} reaction is considered to be the main neutron source responsible for the production of heavy nuclides (from {Sr} to {Bi}) through slow n-capture nucleosynthesis (s-process) at low temperatures during the asymptotic giant branch phase of low-mass stars (≲ 3{--}4 {M}⊙ , or LMSs). In recent years, several direct and indirect measurements have been carried out to determine the cross section at the energies of astrophysical interest (around 190+/- 40 {keV}). However, they yield inconsistent results that cause a highly uncertain reaction rate and affect the neutron release in LMSs. In this work we have combined two indirect approaches, the asymptotic normalization coefficient and the Trojan horse method, to unambiguously determine the absolute value of the {}13{{C}}{(α ,n)}16{{O}} astrophysical factor. With these, we have determined a very accurate reaction rate to be introduced into astrophysical models of s-process nucleosynthesis in LMSs. Calculations using this recommended rate have shown limited variations in the production of those neutron-rich nuclei (with 86≤slant A≤slant 209) that receive contribution only by slow neutron captures.

  14. Quantum radar cross sections

    NASA Astrophysics Data System (ADS)

    Lanzagorta, Marco

    2010-06-01

    The radar cross section σC is an objective measure of the "radar visibility" of an object. As such, σC is an important concept for the correct characterization of the operational performance of radar systems. Furthermore, σC is equally essential for the design and development of stealth weapon systems and platforms. Recent years have seen the theoretical development of quantum radars, that is, radars that operate with a small number of photons. In this regime, the radar-target interaction is described through photon-atom scattering processes governed by the laws of quantum electrodynamics. As such, it is theoretically inconsistent to use the same σC to characterize the performance of a quantum radar. In this paper we define a quantum radar cross section σQ based on quantum electrodynamics and interferometric considerations. We discuss the theoretical challenges of defining σQ, as well as computer simulations of σC and σQ for simple targets.

  15. Photoionization of zinc by TDLDA calculations

    NASA Astrophysics Data System (ADS)

    Stener, M.; Decleva, P.

    1997-10-01

    Absolute photoionization cross section profiles of Zn have been calculated at TDLDA and LDA level, employing a very accurate B-spline basis set and the modified Sternheimer approach. The van Leeuwen - Baerends exchange correlation potential has been used, since its correct asymptotic behaviour is able to support virtual states and describe core-excited resonances. A comparison with available theoretical and experimental data has been performed when possible. The present method has been proven to be robust to analyse wide photon energy regions (from threshold up to 200 eV) and discuss the various shapes of one-electron resonances.

  16. High-Resolution Measurements of Photoionization of Ions Using Synchrotron Radiation

    SciTech Connect

    Aguilar, A.; Covington, A.M.; Emmons, E.D.; Gharaibeh, M.F.; Phaneuf, R.A.; Alvarez, I.; Cisneros, C.; Hinojosa, G.; Dominguez, I.; Ackerman, G.; Bozek, J.D.; Canton, S.; Rude, B.; Sant'Anna, M.M.; Schlachter, A. S.; Folkmann, F.

    2003-08-26

    Measurement of absolute cross sections for photoionization of ions has become feasible by merging a well-collimated ion beam with a monochromatic beam of synchrotron radiation. An electron cyclotron resonance (ECR) ion source permits such measurements to be extended to multiply charged ions, and makes possible systematic studies along isoelectronic sequences. The evolution of atomic spectra along such sequences is commonly studied theoretically, but the predictive ability of the theoretical methods remains largely untested. Absolute cross-section measurements are presented for the first three ionic members of the isoelectronic sequence of nitrogen (O+, F2+ and Ne3+)

  17. International Evaluation of Neutron Cross Section Standards

    NASA Astrophysics Data System (ADS)

    Carlson, A. D.; Pronyaev, V. G.; Smith, D. L.; Larson, N. M.; Chen, Zhenpeng; Hale, G. M.; Hambsch, F.-J.; Gai, E. V.; Oh, Soo-Youl; Badikov, S. A.; Kawano, T.; Hofmann, H. M.; Vonach, H.; Tagesen, S.

    2009-12-01

    Neutron cross section standards are the basis for the determination of most neutron cross sections. They are used for both measurements and evaluations of neutron cross sections. Not many cross sections can be obtained absolutely - most cross sections are measured relative to the cross section standards and converted using evaluations of the standards. The previous complete evaluation of the neutron cross section standards was finished in 1987 and disseminated as the NEANDC/INDC and ENDF/B-VI standards. R-matrix model fits for the light elements and non-model least-squares fits for all the cross sections in the evaluation were the basis of the combined fits for all of the data. Some important reactions and constants are not standards, but they assist greatly in the determination of the standard cross sections and reduce their uncertainties - these data were also included in the combined fits. The largest experimental database used in the evaluation was prepared by Poenitz and included about 400 sets of experimental data with covariance matrices of uncertainties that account for all cross-energy, cross-reaction and cross-material correlations. For the evaluation GMA, a least-squares code developed by Poenitz, was used to fit all types of cross sections (absolute and shape), their ratios, spectrum-averaged cross sections and thermal constants in one full analysis. But, the uncertainties derived in this manner, and especially those obtained in the R-matrix model fits, have been judged to be too low and unrealistic. These uncertainties were substantially increased prior to their release in the recommended data files of 1987. Modified percentage uncertainties were reassigned by the United States Cross Section Evaluation Working Group's Standards Subcommittee for a wide range of energies, and no covariance (or correlation) matrices were supplied at that time. The need to re-evaluate the cross section standards is based on the appearance of a significant amount of precise

  18. New Arsenic Cross Section Calculations

    SciTech Connect

    Kawano, Toshihiko

    2015-03-04

    This report presents calculations for the new arsenic cross section. Cross sections for 73,74,75 As above the resonance range were calculated with a newly developed Hauser-Feshbach code, CoH3.

  19. Photoionization of the cerium isonuclear sequence and cerium endohedral fullerene

    NASA Astrophysics Data System (ADS)

    Habibi, Mustapha

    This dissertation presents an experimental photoionization study of the cerium isonuclear sequence ions in the energy range of the 4d inner-shell giant resonance. In addition, single and double photoionization and photofragmentation cross sections of the cerium endohedral ion Ce C+82 were also measured and studied in the 4d excitation-ionization energy range of cerium. Relative and absolute cross-section measurements were performed at undulator beamline 10.0.1 of the Advanced Light Source (ALS) for nine parent cerium ions: Ce+ - Ce9+. Double-to-single ionization cross-section ratios were measured for photoionization of the endohedral Ce C+82 and empty fullerene C C+82 molecular ions. The merged ion and photon beams technique was used to conduct the experiments. Multiconfiguration Hartree-Fock calculations were performed as an aid to interpret the experimental data. Four Rydberg series for 4d → nf (n ≥ 4) and 4d → np (n ≥ 6) autoionizing excitations were assigned using the quantum defect theory for the Ce3+ photoionization cross section. The experimental data show the collapse of the nf wavefunctions (n ≥ 4) with increasing ionization stage as outer-shell electrons are stripped from the parent ion. The nf orbital collapse occurs partially for Ce2+ and Ce3+ ion and completely for Ce4+, where these wavefunctions penetrate the core region of the ion. A strong contribution to the total oscillator strength was observed in the double and triple photoionization channels for low charge states (Ce +, Ce2+, and Ce3+), whereas most of the 4d excitations of the higher charge states decay by ejection of one electron.

  20. Difference between interaction cross sections and reaction cross sections

    SciTech Connect

    Kohama, Akihisa; Iida, Kei; Oyamatsu, Kazuhiro

    2008-12-15

    We study the validity of the substitution of interaction cross sections for total reaction cross sections for a nucleus incident on a target nucleus at relativistic energies. We show that, for incident stable nuclei, the predicted difference between interaction and total reaction cross sections is large enough to probe the nuclear structure, particularly in a mass region of less than around 40. For analyses of the difference, we construct ''pseudo data'' for the reaction cross sections because empirical data are very limited at high energies. The construction of the pseudo data is based on our assumption that empirically unknown total reaction cross sections are precisely predicted by the phenomenological black-sphere model of nuclei that we developed recently. The comparison with the empirical interaction cross sections suggests a significant difference between the reaction and interaction cross sections for stable projectiles on a carbon target, which is of the order of 0-100 mb.

  1. High efficiency photoionization detector

    DOEpatents

    Anderson, D.F.

    1984-01-31

    A high efficiency photoionization detector is described using tetraaminoethylenes in a gaseous state having a low ionization potential and a relative photoionization cross section which closely matches the emission spectrum of xenon gas. Imaging proportional counters are also disclosed using the novel photoionization detector of the invention. The compound of greatest interest is TMAE which comprises tetrakis(dimethylamino)ethylene which has a measured ionization potential of 5.36 [+-] 0.02 eV, and a vapor pressure of 0.35 torr at 20 C. 6 figs.

  2. High efficiency photoionization detector

    DOEpatents

    Anderson, David F.

    1984-01-01

    A high efficiency photoionization detector using tetraaminoethylenes in a gaseous state having a low ionization potential and a relative photoionization cross section which closely matches the emission spectrum of xenon gas. Imaging proportional counters are also disclosed using the novel photoionization detector of the invention. The compound of greatest interest is TMAE which comprises tetrakis(dimethylamino)ethylene which has a measured ionization potential of 5.36.+-.0.02 eV, and a vapor pressure of 0.35 torr at 20.degree. C.

  3. Merged-beam measurements of absolute cross sections for electron-impact excitation of S{sup 4+} (3s{sup 2} {sup 1}S{yields}3s3p {sup 1}P) and S{sup 5+} (3s {sup 2}S{yields}3p {sup 2}P)

    SciTech Connect

    Wallbank, B.; Bannister, M. E.; Krause, H. F.; Chung, Y.-S.; Smith, A. C. H.; Djuric, N.; Dunn, G. H.

    2007-05-15

    Absolute cross sections for electron-impact excitation of the dipole-allowed transitions S{sup 4+} (3s{sup 2} {sup 1}S{yields}3s3p {sup 1}P) and S{sup 5+} (3s {sup 2}S{yields}3p {sup 2}P) were measured near threshold using the merged electron-ion beams energy-loss technique. Although the magnitudes of the measured cross sections are in reasonable agreement with available theoretical data, the experimental data indicate that the contributions of dielectronic resonances in the near-threshold region are underestimated by these calculations.

  4. Absolute cross sections of electron attachment to molecular clusters. Part II: Formation of (H2O) N - , (N2O) N - , and (N2) N -

    NASA Astrophysics Data System (ADS)

    Vostrikov, A. A.; Dubov, D. Yu.

    2006-12-01

    Absolute cross sections σ-( E, N) of electron attachment to clusters (H2O) N , (N2O) N , and (N2) N for varying electron energy E and cluster size N are measured by using crossed electron and cluster beams in a vacuum. Continua of σ-( E) are found that correlate well with the functions of electron impact excitation of molecules’ internal degrees of freedom. The electron is attached through its solvation in a cluster. In the formation of (H2O){/N -}, (N2O){/N -}, and (N2){/N -}, the curves σ-( N) have a well-defined threshold because of a rise in the electron thermalization and solvation probability with N. For (H2O)900, (N2O)350, and (N2)260 clusters at E = 0.2 eV, the energy losses by the slow electron in the cluster are estimated as 3.0 × 107, 2.7 × 107, and 6.0 × 105 eV/m, respectively. It is found that the growth of σ- with N is the fastest for (H2O) N and (N2) N clusters at E → 0 as a result of polarization capture of the s-electron. Specifically, at E = 0.1 eV and N = 260, σ- = 3.0 × 10-13 cm2 for H2O clusters, 8.0 × 10-14 cm2 for N2O clusters, and 1.4 × 10-15 cm2 for N2 clusters; at E = 11 eV, σ- = 9.0 × 10-16 cm2 for (H2O)200 clusters, 2.4 × 10-14 cm2 for (N2O)350 clusters, and 5.0 × 10-17 cm2 for (N2)260 clusters; finally, at E = 30 eV, σ- = 3.6 × 10-17 cm2 for (N2O)10 clusters and 3.0 × 10-17 cm2 for (N2)125 clusters.

  5. Photoionizing Trapped Highly Charged Ions with Synchrotron Radiation

    SciTech Connect

    Crespo, J R; Simon, M; Beilmann, C; Rudolph, J; Steinbruegge, R; Eberle, S; Schwarz, M; Baumann, T; Schmitt, B; Brunner, F; Ginzel, R; Klawitter, R; Kubicek, K; Epp, S; Mokler, P; Maeckel, V; Ullrich, J; Brown, G V; Graf, A; Leutenegger, M; Beiersdorfer, P; Behar, E; Follath, R; Reichardt, G; Schwarzkopf, O

    2011-09-12

    Photoabsorption by highly charged ions plays an essential role in astrophysical plasmas. Diagnostics of photoionized plasmas surrounding binary systems rely heavily on precise identification of absorption lines and on the knowledge of their cross sections and widths. Novel experiments using an electron beam ion trap, FLASH EBIT, in combination with monochromatic synchrotron radiation allow us to investigate ions in charge states hitherto out of reach. Trapped ions can be prepared in any charge state at target densities sufficient to measure absorption cross sections below 0.1 Mb. The results benchmark state-of-the-art predictions of the transitions wavelengths, widths, and absolute cross sections. Recent high resolution results on Fe{sup 14+}, Fe{sup 15+}, and Ar{sup 12+} at photon energies up to 1 keV are presented.

  6. Radar cross section of insects

    NASA Astrophysics Data System (ADS)

    Riley, J. R.

    1985-02-01

    X-band measurements of radar cross section as a function of the angle between insect body axis and the plane of polarization are presented. A finding of particular interest is that in larger insects, maximum cross section occurs when the E-vector is perpendicular to the body axis. A new range of measurements on small insects (aphids, and planthoppers) is also described, and a comprehensive summary of insect cross-section data at X-band is given.

  7. XCOM: Photon Cross Sections Database

    National Institute of Standards and Technology Data Gateway

    SRD 8 XCOM: Photon Cross Sections Database (Web, free access)   A web database is provided which can be used to calculate photon cross sections for scattering, photoelectric absorption and pair production, as well as total attenuation coefficients, for any element, compound or mixture (Z <= 100) at energies from 1 keV to 100 GeV.

  8. Differential cross sections for positron-xenon elastic scattering

    SciTech Connect

    Marler, J. P.; Surko, C. M.; McEachran, R. P.; Stauffer, A. D.

    2006-06-15

    Absolute measurements of differential cross sections for the elastic scattering of positrons from xenon are made at 2, 5 and 8 eV using a trap-based beam and the technique of measuring scattering cross sections in a strong magnetic field. Calculations are carried out using the relativistic Dirac equations with a static plus polarization potential. Generally good absolute agreement is found between experiment and theory.

  9. Ratios of dijet production cross sections as a function of the absolute difference in rapidity between jets in proton-proton collisions at sqrt{s} = 7 TeV

    NASA Astrophysics Data System (ADS)

    Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; Adam, W.; Bergauer, T.; Dragicevic, M.; Erö, J.; Fabjan, C.; Friedl, M.; Frühwirth, R.; Ghete, V. M.; Hammer, J.; Hoch, M.; Hörmann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Krammer, M.; Liko, D.; Mikulec, I.; Pernicka, M.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schöfbeck, R.; Strauss, J.; Taurok, A.; Teischinger, F.; Wagner, P.; Waltenberger, W.; Walzel, G.; Widl, E.; Wulz, C.-E.; Mossolov, V.; Shumeiko, N.; Suarez Gonzalez, J.; Bansal, S.; Benucci, L.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Luyckx, S.; Maes, T.; Mucibello, L.; Ochesanu, S.; Roland, B.; Rougny, R.; Selvaggi, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.; Blekman, F.; Blyweert, S.; D'Hondt, J.; Gonzalez Suarez, R.; Kalogeropoulos, A.; Maes, M.; Olbrechts, A.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.; Charaf, O.; Clerbaux, B.; De Lentdecker, G.; Dero, V.; Gay, A. P. R.; Hammad, G. H.; Hreus, T.; Léonard, A.; Marage, P. E.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wickens, J.; Adler, V.; Beernaert, K.; Cimmino, A.; Costantini, S.; Garcia, G.; Grunewald, M.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Ocampo Rios, A. A.; Ryckbosch, D.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Vanelderen, L.; Verwilligen, P.; Walsh, S.; Yazgan, E.; Zaganidis, N.; Basegmez, S.; Bruno, G.; Ceard, L.; De Favereau De Jeneret, J.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Grégoire, G.; Hollar, J.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Schul, N.; Beliy, N.; Caebergs, T.; Daubie, E.; Alves, G. A.; Correa Martins Junior, M.; De Jesus Damiao, D.; Martins, T.; Pol, M. E.; Souza, M. H. G.; Aldá Júnior, W. L.; Carvalho, W.; Custódio, A.; Da Costa, E. M.; De Oliveira Martins, C.; Fonseca De Souza, S.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Oguri, V.; Prado Da Silva, W. L.; Santoro, A.; Silva Do Amaral, S. M.; Soares Jorge, L.; Sznajder, A.; Anjos, T. S.; Bernardes, C. A.; Dias, F. A.; Fernandez Perez Tomei, T. R.; Gregores, E. M.; Lagana, C.; Marinho, F.; Mercadante, P. G.; Novaes, S. F.; Padula, Sandra S.; Genchev, V.; Iaydjiev, P.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Tcholakov, V.; Trayanov, R.; Vutova, M.; Dimitrov, A.; Hadjiiska, R.; Karadzhinova, A.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, J.; Wang, J.; Wang, X.; Wang, Z.; Xiao, H.; Xu, M.; Zang, J.; Zhang, Z.; Asawatangtrakuldee, C.; Ban, Y.; Guo, S.; Guo, Y.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Teng, H.; Wang, S.; Zhu, B.; Zou, W.; Cabrera, A.; Gomez Moreno, B.; Osorio Oliveros, A. F.; Sanabria, J. C.; Godinovic, N.; Lelas, D.; Plestina, R.; Polic, D.; Puljak, I.; Antunovic, Z.; Dzelalija, M.; Kovac, M.; Brigljevic, V.; Duric, S.; Kadija, K.; Luetic, J.; Morovic, S.; Attikis, A.; Galanti, M.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Finger, M.; Finger, M.; Assran, Y.; Ellithi Kamel, A.; Khalil, S.; Mahmoud, M. A.; Radi, A.; Hektor, A.; Kadastik, M.; Müntel, M.; Raidal, M.; Rebane, L.; Tiko, A.; Azzolini, V.; Eerola, P.; Fedi, G.; Voutilainen, M.; Czellar, S.; Härkönen, J.; Heikkinen, A.; Karimäki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampén, T.; Lassila-Perini, K.; Lehti, S.; Lindén, T.; Luukka, P.; Mäenpää, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Ungaro, D.; Wendland, L.; Banzuzi, K.; Korpela, A.; Tuuva, T.; Sillou, D.; Besancon, M.; Choudhury, S.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; Hamel de Monchenault, G.; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Rander, J.; Rosowsky, A.; Shreyber, I.; Titov, M.; Baffioni, S.; Beaudette, F.; Benhabib, L.; Bianchini, L.; Bluj, M.; Broutin, C.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dobrzynski, L.; Elgammal, S.; Granier de Cassagnac, R.; Haguenauer, M.; Miné, P.; Mironov, C.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Thiebaux, C.; Veelken, C.; Zabi, A.; Agram, J.-L.; Andrea, J.; Bloch, D.; Bodin, D.; Brom, J.-M.; Cardaci, M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Ferro, C.; Fontaine, J.-C.; Gelé, D.; Goerlach, U.; Juillot, P.; Karim, M.; Le Bihan, A.-C.; Van Hove, P.; Fassi, F.; Mercier, D.; Baty, C.; Beauceron, S.; Beaupere, N.; Bedjidian, M.; Bondu, O.; Boudoul, G.; Boumediene, D.; Brun, H.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Falkiewicz, A.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Le Grand, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sordini, V.; Tosi, S.; Tschudi, Y.; Verdier, P.; Viret, S.

    2012-11-01

    A study of dijet production in proton-proton collisions was performed at sqrt{s}=7 TeV for jets with p T>35 GeV and | y|<4.7 using data collected with the CMS detector at the LHC in 2010. Events with at least one pair of jets are denoted as "inclusive". Events with exactly one pair of jets are called "exclusive". The ratio of the cross section of all pairwise combinations of jets to the exclusive dijet cross section as a function of the rapidity difference between jets |Δ y| is measured for the first time up to |Δ y|=9.2. The ratio of the cross section for the pair consisting of the most forward and the most backward jet from the inclusive sample to the exclusive dijet cross section is also presented. The predictions of the Monte Carlo event generators pythia6 and pythia8 agree with the measurements. In both ratios the herwig++ generator exhibits a more pronounced rise versus |Δ y| than observed in the data. The BFKL-motivated generators cascade and hej+ariadne predict for these ratios a significantly stronger rise than observed.

  10. L -shell photoionization of M n5 + to M n8 + ions

    NASA Astrophysics Data System (ADS)

    Blancard, C.; Cubaynes, D.; Guilbaud, S.; Bizau, J.-M.

    2017-07-01

    Resonant photoionization cross sections of M nn + (n =5 to 8) ions are measured in absolute values in the photon energy range of the 2 p →3 d transitions (645 -690 eV ) using a merged-beams setup at the SOLEIL synchrotron radiation facility. The experimental cross sections are compared to calculations we performed using a multiconfiguration Dirac-Fock code and the opas code dedicated to radiative opacity calculations of hot and dense plasmas. Both calculations reproduce the measurements well.

  11. Absolute cross section for the reaction /sup 3/H(p,. gamma. /sub 0/)/sup 4/He and a review of /sup 4/He(. gamma. , p/sub 0/)/sup 3/H measurements

    SciTech Connect

    Calarco, J.R.; Hanna, S.S.; Chang, C.C.; Diener, E.M.; Kuhlmann, E.; Fisher, G.A.

    1983-08-01

    Accurate differential cross sections have been measured at 90/sup 0/ for the reaction /sup 3/H(p,..gamma..)/sup 4/He at E/sub p/ = 8.34 and 13.6 MeV. Previously published results for both /sup 3/H(p,..gamma..)/sup 4/He and /sup 4/He(..gamma..,p)/sup 3/H are reviewed and compared with the present data. The theoretical implications of the results are briefly discussed.

  12. Photoionization and Recombination

    NASA Technical Reports Server (NTRS)

    Nahar, Sultana N.

    2000-01-01

    Theoretically self-consistent calculations for photoionization and (e + ion) recombination are described. The same eigenfunction expansion for the ion is employed in coupled channel calculations for both processes, thus ensuring consistency between cross sections and rates. The theoretical treatment of (e + ion) recombination subsumes both the non-resonant recombination ("radiative recombination"), and the resonant recombination ("di-electronic recombination") processes in a unified scheme. In addition to the total, unified recombination rates, level-specific recombination rates and photoionization cross sections are obtained for a large number of atomic levels. Both relativistic Breit-Pauli, and non-relativistic LS coupling, calculations are carried out in the close coupling approximation using the R-matrix method. Although the calculations are computationally intensive, they yield nearly all photoionization and recombination parameters needed for astrophysical photoionization models with higher precision than hitherto possible, estimated at about 10-20% from comparison with experimentally available data (including experimentally derived DR rates). Results are electronically available for over 40 atoms and ions. Photoionization and recombination of He-, and Li-like C and Fe are described for X-ray modeling. The unified method yields total and complete (e+ion) recombination rate coefficients, that can not otherwise be obtained theoretically or experimentally.

  13. Cross sections at hadron colliders

    SciTech Connect

    Paige, F.E.

    1982-01-01

    The predicted cross sections are given for new Z'/sup 0/ bosons, for the Drell-Yan continuum of ..mu../sup +/..mu../sup -/ pairs, for high p/sub T/ hadron jets, for high p/sub T/ single photons, and for the associated production of heavy quarks. These processes have been selected not to cover the most interesting physics, but to provide a representative selection of cross sections for which to compare various energies and luminosities.

  14. Experimental and theoretical investigations on photoabsorption and photoionization of trimethylphosphate in the vacuum-ultraviolet energy range

    NASA Astrophysics Data System (ADS)

    Homem, M. G. P.; López-Castillo, A.; Barbatti, M.; Rosa, L. F. S.; Iza, P.; Cavasso-Filho, R. L.; Farenzena, L. S.; Lee, M. T.; Iga, I.

    2012-11-01

    In this work, we report a joint experimental-theoretical investigation on interaction of vacuum-ultraviolet radiation with trimethylphosphate (TMP) molecule (C3H9O4P) in gas phase. This species together with tetrahydrofuran (THF) are model compounds of deoxyribose nucleic acids (DNA)/ribose nucleic acids (RNA) backbone. Absolute photoabsorption cross sections (σa) and ionization yields (η) are measured using the double-ion-chamber technique in the 11.0-21.45 eV energy range. Photoionization (σi) and neutral-decay (σn) cross sections in absolute scale are also derived. Moreover, theoretical photoabsorption cross sections are calculated using the time-dependent density functional theory from the excitation threshold up to 16 eV. Good agreement between the present calculated and experimental photoabsorption cross sections in the 11.0-14.5 eV range is encouraging. Also, the present measured data of σa and σi for TMP are about 1.3 and 1.5 times of those of THF, respectively. Thus, the experimental evidences that the majority of strand breaks being located at sugar rings in the irradiated DNA/RNA backbone moiety may be induced by a possible migration of the hole, initially created at phosphate group, to the linked sugar groups. Finally, absolute partial photoionization cross sections are derived from the experimental time-of-flight mass spectra.

  15. Experimental and theoretical investigations on photoabsorption and photoionization of trimethylphosphate in the vacuum-ultraviolet energy range.

    PubMed

    Homem, M G P; López-Castillo, A; Barbatti, M; Rosa, L F S; Iza, P; Cavasso-Filho, R L; Farenzena, L S; Lee, M T; Iga, I

    2012-11-14

    In this work, we report a joint experimental-theoretical investigation on interaction of vacuum-ultraviolet radiation with trimethylphosphate (TMP) molecule (C(3)H(9)O(4)P) in gas phase. This species together with tetrahydrofuran (THF) are model compounds of deoxyribose nucleic acids (DNA)/ribose nucleic acids (RNA) backbone. Absolute photoabsorption cross sections (σ(a)) and ionization yields (η) are measured using the double-ion-chamber technique in the 11.0-21.45 eV energy range. Photoionization (σ(i)) and neutral-decay (σ(n)) cross sections in absolute scale are also derived. Moreover, theoretical photoabsorption cross sections are calculated using the time-dependent density functional theory from the excitation threshold up to 16 eV. Good agreement between the present calculated and experimental photoabsorption cross sections in the 11.0-14.5 eV range is encouraging. Also, the present measured data of σ(a) and σ(i) for TMP are about 1.3 and 1.5 times of those of THF, respectively. Thus, the experimental evidences that the majority of strand breaks being located at sugar rings in the irradiated DNA/RNA backbone moiety may be induced by a possible migration of the hole, initially created at phosphate group, to the linked sugar groups. Finally, absolute partial photoionization cross sections are derived from the experimental time-of-flight mass spectra.

  16. Atomic photoionization experiment by harmonic-generation spectroscopy

    NASA Astrophysics Data System (ADS)

    Frolov, M. V.; Sarantseva, T. S.; Manakov, N. L.; Fulfer, K. D.; Wilson, B. P.; Troß, J.; Ren, X.; Poliakoff, E. D.; Silaev, A. A.; Vvedenskii, N. V.; Starace, Anthony F.; Trallero-Herrero, C. A.

    2016-03-01

    Measurements of the high-order-harmonic generation yield of the argon (Ar) atom driven by a strong elliptically polarized laser field are shown to completely determine the field-free differential photoionization cross section of Ar, i.e., the energy dependence of both the angle-integrated photoionization cross section and the angular distribution asymmetry parameter.

  17. Temperature-dependent absorption cross sections for hydrogen peroxide vapor

    NASA Technical Reports Server (NTRS)

    Nicovich, J. M.; Wine, P. H.

    1988-01-01

    Relative absorption cross sections for hydrogen peroxide vapor were measured over the temperature ranges 285-381 K for lambda = 230 nm-295 nm and 300-381 K for lambda = 193 nm-350 nm. The well established 298 K cross sections at 202.6 and 228.8 nm were used as an absolute calibration. A significant temperature dependence was observed at the important tropospheric photolysis wavelengths lambda over 300 nm. Measured cross sections were extrapolated to lower temperatures, using a simple model which attributes the observed temperature dependence to enhanced absorption by molecules possessing one quantum of O-O stretch vibrational excitation. Upper tropospheric photodissociation rates calculated using the extrapolated cross sections are about 25 percent lower than those calculated using currently recommended 298 K cross sections.

  18. Temperature-dependent absorption cross sections for hydrogen peroxide vapor

    NASA Astrophysics Data System (ADS)

    Nicovich, J. M.; Wine, P. H.

    1988-03-01

    Relative absorption cross sections for hydrogen peroxide vapor were measured over the temperature ranges 285-381 K for lambda = 230 nm-295 nm and 300-381 K for lambda = 193 nm-350 nm. The well established 298 K cross sections at 202.6 and 228.8 nm were used as an absolute calibration. A significant temperature dependence was observed at the important tropospheric photolysis wavelengths lambda over 300 nm. Measured cross sections were extrapolated to lower temperatures, using a simple model which attributes the observed temperature dependence to enhanced absorption by molecules possessing one quantum of O-O stretch vibrational excitation. Upper tropospheric photodissociation rates calculated using the extrapolated cross sections are about 25 percent lower than those calculated using currently recommended 298 K cross sections.

  19. Accurate Cross Sections for Microanalysis

    PubMed Central

    Rez, Peter

    2002-01-01

    To calculate the intensity of x-ray emission in electron beam microanalysis requires a knowledge of the energy distribution of the electrons in the solid, the energy variation of the ionization cross section of the relevant subshell, the fraction of ionizations events producing x rays of interest and the absorption coefficient of the x rays on the path to the detector. The theoretical predictions and experimental data available for ionization cross sections are limited mainly to K shells of a few elements. Results of systematic plane wave Born approximation calculations with exchange for K, L, and M shell ionization cross sections over the range of electron energies used in microanalysis are presented. Comparisons are made with experimental measurement for selected K shells and it is shown that the plane wave theory is not appropriate for overvoltages less than 2.5 V. PMID:27446747

  20. Two-Particle Coulomb Green Function Method with Projected Potential: Application to He Double Photoionization

    NASA Astrophysics Data System (ADS)

    Argenti, Luca; Colle, Renato

    2009-08-01

    A new method to compute fully differential double photoionization cross sections of atoms has been devised and fully developed for two-electron systems. The method exploits the Green function for two noninteracting electrons in the field of a nuclear charge to infer the effects of the residual potential projected on a set of L2-basis functions. Test calculations on helium at 100 eV excess energy indicate that, as long as the relevant part of the interaction potential is accounted for, the fully differential cross sections calculated in acceleration and velocity gauges converge in absolute value and reproduce measured angular distributions with a tunable accuracy. Generalization of the method to treat double photoionization of many-electron atoms is sketched.

  1. Two-particle coulomb Green function method with projected potential: application to He double photoionization.

    PubMed

    Argenti, Luca; Colle, Renato

    2009-12-31

    A new method to compute fully differential double photoionization cross sections of atoms has been devised and fully developed for two-electron systems. The method exploits the Green function for two noninteracting electrons in the field of a nuclear charge to infer the effects of the residual potential projected on a set of L(2)-basis functions. Test calculations on helium at 100 eV excess energy indicate that, as long as the relevant part of the interaction potential is accounted for, the fully differential cross sections calculated in acceleration and velocity gauges converge in absolute value and reproduce measured angular distributions with a tunable accuracy. Generalization of the method to treat double photoionization of many-electron atoms is sketched.

  2. Diffusion cross sections for potassium ? and ? levels in rare gases

    NASA Astrophysics Data System (ADS)

    Yahyaei-Moayyed, F.; Hickman, A. P.; Streater, A. D.

    1996-02-01

    We have used a light-induced drift (LID) experiment to determine ratios of cross sections for diffusion of potassium in the excited 0953-4075/29/3/011/img3, 0953-4075/29/3/011/img4 and the ground 0953-4075/29/3/011/img5 levels in five rare gases. The measured ratios are combined with the ground-state cross sections and statistically averaged excited cross sections, available from a previously reported light induced diffusive pulling experiment, to obtain the absolute cross sections for individual fine structure levels. We also report calculated cross sections based on available potential curves and a coupled-channel theory. Rough qualitative agreement is generally found between the absolute cross sections inferred from experiment and the theoretical values. The light-induced drift experiments, however, measure ratios of cross section differences that are highly sensitive to the potential curves. It is found that the available potential curves are not adequate for predicting these measured ratios.

  3. High-efficiency photoionization detector

    SciTech Connect

    Anderson, D.F.

    1981-05-12

    A high efficiency photoionization detector using tetraaminoethylenes in a gaseous state having a low ionization potential and a relative photoionization cross section which closely matches the emission spectrum of xenon gas. Imaging proportional counters are also disclosed using the novel photoionization detector of the invention. The compound of greatest interest is TMAE which comprises tetrakis(dimethylamino)ethylene which has a measured ionization potential of 5.36 +- 0.02 eV, and a vapor pressure of 0.35 torr at 20/sup 0/C.

  4. Neutrino cross-sections: Experiments

    SciTech Connect

    Sánchez, F.

    2015-07-15

    Neutrino-nucleus cross-sections are as of today the main source of systematic errors for oscillation experiments together with neutrino flux uncertainties. Despite recent experimental and theoretical developments, future experiments require even higher precisions in their search of CP violation. We will review the experimental status and explore possible future developments required by next generation of experiments.

  5. Photoneutron cross sections for Au

    SciTech Connect

    Itoh, O.; Utsunomiya, H.; Akimune, H.; Yamagata, T.; Kondo, T.; Kamata, M.; Toyokawa, H.; Harada, H.; Kitatani, F.; Goko, S.; Nair, C.; Lui, Y.-W.

    2011-10-28

    Photoneutron cross sections were measured for Au in the entire energy range of the ({gamma},n) channel based on a direct neutron-counting technique with quasimonochromatic {gamma} rays produced in inverse Compton-scattering of laser photons with relativistic electrons. We present results of the measurement in comparison with the past data.

  6. A rare gas optics-free absolute photon flux and energy analyzer to provide absolute photoionization rates of inflowing interstellar neutrals

    NASA Technical Reports Server (NTRS)

    Judge, Darrell L.

    1994-01-01

    A prototype spectrometer has been developed for space applications requiring long term absolute EUV photon flux measurements. The energy spectrum of the incoming photons is transformed directly into an electron energy spectrum by taking advantage of the photoelectric effect in one of several rare gases at low pressures. Using an electron energy spectrometer, followed by an electron multiplier detector, pulses due to individual electrons are counted. The overall efficiency of this process can be made essentially independent of gain drifts in the signal path, and the secular degradation of optical components which is often a problem in other techniques is avoided. A very important feature of this approach is its freedom from the problem of overlapping spectral orders that plagues grating EUV spectrometers. An instrument with these features has not been flown before, but is essential to further advances in our understanding of solar EUV flux dynamics, and the coupled dynamics of terrestrial and planetary atmospheres. The detailed characteristics of this optics-free spectrometer are presented in the publications section.

  7. Photoelectron wave function in photoionization: Plane wave or Coulomb wave? [Does photoionization of neutral targets produce Coulomb or plane waves?

    DOE PAGES

    Gozem, Samer; Gunina, Anastasia O.; Ichino, Takatoshi; ...

    2015-10-28

    The calculation of absolute total cross sections requires accurate wave functions of the photoelectron and of the initial and final states of the system. The essential information contained in the latter two can be condensed into a Dyson orbital. We employ correlated Dyson orbitals and test approximate treatments of the photoelectron wave function, that is, plane and Coulomb waves, by comparing computed and experimental photoionization and photodetachment spectra. We find that in anions, a plane wave treatment of the photoelectron provides a good description of photodetachment spectra. For photoionization of neutral atoms or molecules with one heavy atom, the photoelectronmore » wave function must be treated as a Coulomb wave to account for the interaction of the photoelectron with the +1 charge of the ionized core. For larger molecules, the best agreement with experiment is often achieved by using a Coulomb wave with a partial (effective) charge smaller than unity. This likely derives from the fact that the effective charge at the centroid of the Dyson orbital, which serves as the origin of the spherical wave expansion, is smaller than the total charge of a polyatomic cation. Finally, the results suggest that accurate molecular photoionization cross sections can be computed with a modified central potential model that accounts for the nonspherical charge distribution of the core by adjusting the charge in the center of the expansion.« less

  8. Photoionization of atoms. Final report, April 1, 1976-March 30, 1981

    SciTech Connect

    Samson, J.A.R.; Starace, A.F.

    1981-11-01

    There were two main goals in the experimental study of photoionization. One was to provide accurate data on the results of photon-atom collisions, studying the absolute probability for ejecting electrons from specific orbitals and determining their angular distributions. Also of interest was the probability for one photon to eject two or more electrons. Another goal was to make measurements of specific interactions that would provide sensitive tests for the various theoretical approximations used in calculating photoionization cross sections. To achieve these two goals, care was taken in the selection of the various experiments and in the use of the most appropriate and sophisticated equipment. For example, the techniques of Photoelectron Spectroscopy, Photoionization - Mass Spectrometry, and Synchrotron radiation were used in many of the experiments.

  9. Cross Sections for Planetary Escape

    NASA Astrophysics Data System (ADS)

    Tully, C.

    2001-05-01

    Energetic charged-particle bombardment, dissociative recombination and photodissociation processes produce energetic recoil atoms which heat the thermosphere and can lead to escape from a planet affecting the evolution of the atmosphere. In describing these processes by Monte Carlo methods, many of the critical cross sections are not available in the energy range of interest, a few eV to 1 keV. Here we present our recent results for elastic collision and collisional dissociation cross sections relevant to Titan, Triton, Europa and the terrestrial planets [1,2]. Elastic and diffusion cross sections were calculated using both quantum mechanical techniques and the semiclassical JWKB approximation for the collision of ground state oxygen atoms in the energy range 1-10eV [2]. This involved calculation of phase shifts for each of the 18 molecular energy states of O2 which separate to two ground state O atoms. For an O thermosphere the total elastic cross section is close to that typically assumed but the escape depths are shown to be larger than those typically used. Dissociation cross sections of N + N2 were calculated using a semiclassical method, in the energy range 0-30eV. This required treating the vibrational motion quantum mechanically while the rotational and the relative translational motion were treated classically. The evolution of the system was calculated by simultaneous propagation of the classical as well as the quantal degrees of freedom. The solution to the classical part was carried out by solving Hamilton equations of motion using an effective London-Eyring-Polanyi-Sato potential energy surface, calculated by Laganá et al [3]. Propagation of the quantal wavefunction was carried out by solving the time dependent Schrödinger equation using the split operator technique with the help of the fast fourier transform which was used to calculate the second derivatives arising from the kinetic energy operator. This work was supported by NASA's Planetary

  10. Partial (gamma)-Ray Cross Sections for the Reaction 239Pu(n,2n(gamma)i) and the 239Pu(n,2n) Cross Section

    SciTech Connect

    Beacker, J.A.; Bernstein, L.A.; Younes, W.; McNabb, D.P.; Garrett, P.E.; Archer, D.; McGrath, C.A.; Stoyer, M.A.; Chen, H.; Ormand, W.E.; Nelson, R.O.; Chadwick, M.B.; Johns, G.D.; Drake, D.; Young, P.G.; Devlin, M.; Fotiades, N.; Wilburn, W.S.

    2001-09-14

    Absolute partial {gamma}-ray cross sections for production of discrete {gamma} rays in the {sup 239}Pu(n,2n{gamma}i){sup 238}Pu reaction have been measured. The experiments were performed at LANSCE/WNR on the 60R flight line. Reaction {gamma}-rays were measured using the large-scale Compton-suppressed array of Ge detectors, GEANIE. The motivation for this experiment, an overview of the partial {gamma}-ray cross-section measurement, and an introduction to the main experimental issues will be presented. The energy resolution of the Ge detectors allowed identification of reaction {gamma} rays above the background of sample radioactivity and fission {gamma} rays. The use of planar Ge detectors with their reduced sensitivity to neutron interactions and improved line shape was also important to the success of this experiment. Absolute partial {gamma}-ray cross sections are presented for the 6{sub 1}{sup +} {yields} 4{sub 1}{sup +} member of the ground state rotational band in {sup 238}Pu, together with miscellaneous other {gamma}-ray partial cross sections. The n,2n reaction cross section shape and magnitude as a function of neutron energy was extracted from these partial cross sections using nuclear modeling (enhanced Hauser-Feshbach) to relate partial {gamma}-ray cross sections to the n,2n cross section. The critical nuclear modeling issue is the ratio of a partial cross section to the reaction channel cross section, and not the prediction of the absolute magnitude.

  11. Photoionization Efficiencies of Five Polycyclic Aromatic Hydrocarbons.

    PubMed

    Johansson, K Olof; Campbell, Matthew F; Elvati, Paolo; Schrader, Paul E; Zádor, Judit; Richards-Henderson, Nicole K; Wilson, Kevin R; Violi, Angela; Michelsen, Hope A

    2017-06-15

    We have measured photoionization-efficiency curves for pyrene, fluoranthene, chrysene, perylene, and coronene in the photon energy range of 7.5-10.2 eV and derived their photoionization cross-section curves in this energy range. All measurements were performed using tunable vacuum ultraviolet (VUV) radiation generated at the Advanced Light Source synchrotron at Lawrence Berkeley National Laboratory. The VUV radiation was used for photoionization, and detection was performed using a time-of-flight mass spectrometer. We measured the photoionization efficiency of 2,5-dimethylfuran simultaneously with those of pyrene, fluoranthene, chrysene, perylene, and coronene to obtain references of the photon flux during each measurement from the known photoionization cross-section curve of 2,5-dimethylfuran.

  12. Cross sections and reaction rates of relevance to aeronomy

    SciTech Connect

    Fox, J.L. )

    1991-01-01

    Experimental and theoretical data relevant to models and measurements of the chemical and thermal structures and luminosity of the thermospheres of the earth and planets published during the last four years are surveyed. Among chemical processes, attention is given to ion-molecule reactions, dissociative recombination of molecular ions, and reactions between neutral species. Both reactions between ground state species and species in excited states are considered, including energy transfer and quenching. Measured and calculated cross sections for interactions of solar radiation with atmospheric species, such as photoabsorption, photoionization, and photodissociation and related processes are surveyed.

  13. Simultaneous evaluation of interrelated cross sections by generalized least-squares and related data file requirements

    SciTech Connect

    Poenitz, W.P.

    1984-10-25

    Though several cross sections have been designated as standards, they are not basic units and are interrelated by ratio measurements. Moreover, as such interactions as /sup 6/Li + n and /sup 10/B + n involve only two and three cross sections respectively, total cross section data become useful for the evaluation process. The problem can be resolved by a simultaneous evaluation of the available absolute and shape data for cross sections, ratios, sums, and average cross sections by generalized least-squares. A data file is required for such evaluation which contains the originally measured quantities and their uncertainty components. Establishing such a file is a substantial task because data were frequently reported as absolute cross sections where ratios were measured without sufficient information on which reference cross section and which normalization were utilized. Reporting of uncertainties is often missing or incomplete. The requirements for data reporting will be discussed.

  14. Partial dissociative emission cross sections and product state distributions of the resulting photofragments

    NASA Astrophysics Data System (ADS)

    Picconi, David; Grebenshchikov, Sergy Yu.

    2016-12-01

    This paper relates the partial cross section of a continuous optical emission into a given scattering channel of the lower electronic state to the photofragment population. This allows one to infer partial emission cross sections 'non-optically' from product state distributions; in computations, explicit construction of exact scattering states is therefore avoided. Applications to the emission spectra of NaI, CO2, and pyrrole are given. It is also demonstrated that a similar relationship holds between partial cross sections of dissociative photoionization and distributions of ionic fragments over final product channels.

  15. Electron-Impact Ionization Cross Section Database

    National Institute of Standards and Technology Data Gateway

    SRD 107 Electron-Impact Ionization Cross Section Database (Web, free access)   This is a database primarily of total ionization cross sections of molecules by electron impact. The database also includes cross sections for a small number of atoms and energy distributions of ejected electrons for H, He, and H2. The cross sections were calculated using the Binary-Encounter-Bethe (BEB) model, which combines the Mott cross section with the high-incident energy behavior of the Bethe cross section. Selected experimental data are included.

  16. Photodissociation cross section of ClOOCl at 330 nm.

    PubMed

    Jin, Bing; Chen, I-Cheng; Huang, Wen-Tsung; Lien, Chien-Yu; Guchhait, Nikhil; Lin, Jim J

    2010-04-15

    The photolysis rate of ClOOCl is crucial in the catalytic destruction of polar stratospheric ozone. In this work, we determined the photodissociation cross section of ClOOCl at 330 nm with a molecular beam and with mass-resolved detection. The photodissociation cross section is the product of the absorption cross section and the dissociation quantum yield. We formed an effusive molecular beam of ClOOCl at a nozzle temperature of 200 or 250 K and determined its photodissociation probability by measuring the decrease of the ClOOCl intensity upon laser irradiation. By comparing with a reference molecule (Cl(2)), of which the absorption cross section and dissociation quantum yield are well-known, we determined the absolute photodissociation cross section of ClOOCl at 330 nm to be (2.31 +/- 0.11) x 10(-19) cm(2) at 200 K and (2.47 +/- 0.12) x 10(-19) cm(2) at 250 K. Impurity interference has been a well-recognized problem in conventional spectroscopic studies of ClOOCl; our mass-resolved measurement directly overcomes such a problem. This measurement of the ClOOCl photolysis cross section at 330 nm is particularly useful in constraining its atmospheric photolysis rate, which in the polar stratosphere peaks near this wavelength.

  17. Measurement of the 242Pu neutron capture cross section

    NASA Astrophysics Data System (ADS)

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; Bucher, B.; Bredeweg, T. A.; Baramsai, B.; Couture, A.; Jandel, M.; Mosby, S.; O'Donnell, J. M.; Ullmann, J. L.; Chyzh, A.; Dance Collaboration

    2015-10-01

    Precision (n,f) and (n, γ) cross sections are important for the network calculations of the radiochemical diagnostic chain for the U.S. DOE's Stockpile Stewardship Program. 242Pu(n, γ) cross section is relevant to the network calculations of Pu and Am. Additionally, new reactor concepts have catalyzed considerable interest in the measurement of improved cross sections for neutron-induced reactions on key actinides. To date, little or no experimental data has been reported on 242Pu(n, γ) for incident neutron energy below 50 keV. A new measurement of the 242Pu(n, γ) reaction was performed with the DANCE together with an improved PPAC for fission-fragment detection at LANSCE during FY14. The relative scale of the 242Pu(n, γ) cross section spans four orders of magnitude for incident neutron energies from thermal to ~ 30 keV. The absolute scale of the 242Pu(n, γ) cross section is set according to the measured 239Pu(n,f) resonance at 7.8 eV; the target was spiked with 239Pu for this measurement. The absolute 242Pu(n, γ) neutron capture cross section is ~ 30% higher than the cross section reported in ENDF for the 2.7 eV resonance. Latest results to be reported. Funded by U.S. DOE Contract No. DE-AC52-07NA27344 (LLNL) and DE-AC52-06NA25396 (LANL). U.S. DOE/NNSA Office of Defense Nuclear Nonproliferation Research and Development. Isotopes (ORNL).

  18. Ionisation cross sections of rare-gas atoms by electron impact

    NASA Technical Reports Server (NTRS)

    Krishnakumar, E.; Srivastava, S. K.

    1988-01-01

    A pulsed electron beam and ion extraction method is used to measure normalized values of partial ionization cross sections for rare gases from threshold to 1000 eV. Cross sections obtained for singly ionized species are used to calibrate the mass transmission efficiency of the ion extraction/analyzer/detection system by the relative flow technique, and this mass transmission curve is then used to determine the absolute cross sections of the multiply ionized species. Total ion cross sections are found by summation of the individual partial cross sections with proper weighting for charge.

  19. Neutron cross sections: Book of curves

    SciTech Connect

    McLane, V.; Dunford, C.L.; Rose, P.F.

    1988-01-01

    Neuton Cross Sections: Book of Curves represents the fourth edition of what was previously known as BNL-325, Neutron Cross Sections, Volume 2, CURVES. Data is presented only for (i.e., intergrated) reaction cross sections (and related fission parameters) as a function of incident-neutron energy for the energy range 0.01 eV to 200 MeV. For the first time, isometric state production cross sections have been included. 11 refs., 4 figs.

  20. Photoproduction total cross section and shower development

    NASA Astrophysics Data System (ADS)

    Cornet, F.; García Canal, C. A.; Grau, A.; Pancheri, G.; Sciutto, S. J.

    2015-12-01

    The total photoproduction cross section at ultrahigh energies is obtained using a model based on QCD minijets and soft-gluon resummation and the ansatz that infrared gluons limit the rise of total cross sections. This cross section is introduced into the Monte Carlo system AIRES to simulate extended air showers initiated by cosmic ray photons. The impact of the new photoproduction cross section on common shower observables, especially those related to muon production, is compared with previous results.

  1. Ozone absorption cross section measurements in the Wulf bands

    NASA Technical Reports Server (NTRS)

    Anderson, Stuart M.; Hupalo, Peter; Mauersberger, Konrad

    1993-01-01

    A tandem dual-beam spectrometer has been developed to determine ozone absorption cross sections for 13 selected wavelengths between 750 and 975 nm at room temperature. The increasingly pronounced structure in this region may interfere with atmospheric trace gas transitions that are useful for remote sensing and complicate the measurement of aerosols. Ozone concentrations were determined by absorption at the common HeNe laser transition near 632.8 nm using the absolute cross section reported previously. The overall accuracy of these room temperature measurements is generally better than 2 percent. A synoptic near-IR spectrum scaled to these measurements is employed for comparison with results of previous studies.

  2. SNL RML recommended dosimetry cross section compendium

    SciTech Connect

    Griffin, P.J.; Kelly, J.G.; Luera, T.F.; VanDenburg, J.

    1993-11-01

    A compendium of dosimetry cross sections is presented for use in the characterization of fission reactor spectrum and fluence. The contents of this cross section library are based upon the ENDF/B-VI and IRDF-90 cross section libraries and are recommended as a replacement for the DOSCROS84 multigroup library that is widely used by the dosimetry community. Documentation is provided on the rationale for the choice of the cross sections selected for inclusion in this library and on the uncertainty and variation in cross sections presented by state-of-the-art evaluations.

  3. [Fast neutron cross section measurements

    SciTech Connect

    Knoll, G.F.

    1992-10-26

    From its inception, the Nuclear Data Project at the University of Michigan has concentrated on two major objectives: (1) to carry out carefully controlled nuclear measurements of the highest possible reliability in support of the national nuclear data program, and (2) to provide an educational opportunity for students with interests in experimental nuclear science. The project has undergone a successful transition from a primary dependence on our photoneutron laboratory to one in which our current research is entirely based on a unique pulsed 14 MeV fast neutron facility. The new experimental facility is unique in its ability to provide nanosecond bursts of 14 MeV neutrons under conditions that are clean'' and as scatter-free as possible, and is the only one of its type currently in operation in the United States. It has been designed and put into operation primarily by graduate students, and has met or exceeded all of its important initial performance goals. We have reached the point of its routine operation, and most of the data are now in hand that will serve as the basis for the first two doctoral dissertations to be written by participating graduate students. Our initial results on double differential neutron cross sections will be presented at the May 1993 Fusion Reactor Technology Workshop. We are pleased to report that, after investing several years in equipment assembly and optimization, the project has now entered its data production'' phase.

  4. Photoabsorption cross section of acetylene in the EUV region

    NASA Technical Reports Server (NTRS)

    Wu, C. Y. R.; Judge, D. L.

    1985-01-01

    The measurement of the absolute photoabsorption cross sections of C2H2 in the 175-740 A region by means of a double ionization chamber is reported. The continuum background source is the synchrotron radiation emitted by the Wisconsin 240 MeV electron storage ring. It is found that the cross sections range from 2 to a maximum of 36 Mb. Two new Rydberg series are identified and the cross section data are applied in the analysis of various sum rules. From the rules, it is shown that the data of C2H2 in the 580-1088 A range may be too low, while the measured ionization transition moment may be too high.

  5. Electron impact cross sections for the 2,2P state excitation of lithium

    NASA Technical Reports Server (NTRS)

    Vuskovic, L.; Trajmar, S.; Register, D. F.

    1982-01-01

    Electron impact excitation of the 2p 2P state of Li was studied at 10, 20, 60, 100, 150 and 200 eV. Relative differential cross sections in the angular range 3-120 deg were measured and then normalized to the absolute scale by using the optical f value. Integral and momentum transfer cross sections were obtained by extrapolating the differential cross sections to 0 deg and to 180 deg. The question of normalizing electron-metal-atom collision cross sections in general was examined and the method of normalization to optical f values in particular was investigated in detail. It has been concluded that the extrapolation of the apparent generalized oscillator strength (obtained from the measured differential cross sections) to the zero momentum transfer limit with an expression using even powers of the momentum transfer and normalization of the limit to the optical f value yields reliable absolute cross sections.

  6. An Atomic Photoionization Experiment by Harmonic Generation Spectroscopy

    NASA Astrophysics Data System (ADS)

    Trallero, Carlos; Frolov, Mikhail; Sarantseva, Tatiana S.; Manakov, Nikolay; Fulfer, Kristen D.; Wilson, Benjamin; Troß, Jan; Ren, Xiaoming; Poliakoff, Erwin; Silaev, Alexander A.; Vvedenskii, Nikolay; Starace, Anthony

    2016-05-01

    Measurements of the high-order harmonic generation yield of the argon (Ar) atom driven by a strong elliptically polarized laser field are shown to completely determine the field-free differential photoionization cross section of Ar, i.e., the energy dependence of both the angle-integrated photoionization cross section and the angular distribution asymmetry parameter. NSF EPSCoR Track II Nebraska-Kansas Awards No. 1430519 and No. 1430493.

  7. Validation of Cross Sections for Monte Carlo Simulation of the Photoelectric Effect

    NASA Astrophysics Data System (ADS)

    Han, Min Cheol; Kim, Han Sung; Pia, Maria Grazia; Basaglia, Tullio; Batic, Matej; Hoff, Gabriela; Kim, Chan Hyeong; Saracco, Paolo

    2016-04-01

    Several total and partial photoionization cross section calculations, based on both theoretical and empirical approaches, are quantitatively evaluated with statistical analyses using a large collection of experimental data retrieved from the literature to identify the state of the art for modeling the photoelectric effect in Monte Carlo particle transport. Some of the examined cross section models are available in general purpose Monte Carlo systems, while others have been implemented and subjected to validation tests for the first time to estimate whether they could improve the accuracy of particle transport codes. The validation process identifies Scofield's 1973 non-relativistic calculations, tabulated in the Evaluated Photon Data Library(EPDL), as the one best reproducing experimental measurements of total cross sections. Specialized total cross section models, some of which derive from more recent calculations, do not provide significant improvements. Scofield's non-relativistic calculations are not surpassed regarding the compatibility with experiment of K and L shell photoionization cross sections either, although in a few test cases Ebel's parameterization produces more accurate results close to absorption edges. Modifications to Biggs and Lighthill's parameterization implemented in Geant4 significantly reduce the accuracy of total cross sections at low energies with respect to its original formulation. The scarcity of suitable experimental data hinders a similar extensive analysis for the simulation of the photoelectron angular distribution, which is limited to a qualitative appraisal.

  8. Cross sections for H(-) and Cl(-) production from HCl by dissociative electron attachment

    NASA Technical Reports Server (NTRS)

    Orient, O. J.; Srivastava, S. K.

    1985-01-01

    A crossed target beam-electron beam collision geometry and a quadrupole mass spectrometer have been used to conduct dissociative electron attachment cross section measurements for the case of H(-) and Cl(-) production from HCl. The relative flow technique is used to determine the absolute values of cross sections. A tabulation is given of the attachment energies corresponding to various cross section maxima. Error sources contributing to total errors are also estimated.

  9. Electron Impact Ionization Cross Sections in Rb and Cs.

    NASA Astrophysics Data System (ADS)

    Reddish, T. J.; Lukomski, M.; Sutton, S.; Kedzierski, W.; McConkey, J. W.; Bartschat, K.; Bartlett, P. L.; Stelbovics, A. T.; Bray, I.

    2006-05-01

    We present a new atom trapping technique for determining absolute, total ionisation cross sections (TICS) out of an excited atom. The novel feature of this method is in utilizing Doppler cooling of neutral atoms to determine ionisation cross sections. This fluorescence-monitoring experiment, which is a variant of the `trap loss' technique, has enabled us to obtain the experimental electron impact ionisation cross sections out of the Cs 6^2P3/2 excited state between 7 - 400 eV. New CCC, R-Matrix with Pseudo-States (RMPS), and Born approximation single ionisation cross sections (SICS) are also presented for both the ground and excited states of Cs and Rb, and compared with the available experimental data. The comparison of the results reveals the importance of the autoionisation and multiple ionisation contributions to the TICS. The autoionisation contribution appears to be substantial for ionisation out of the Cs 6^2P and Rb 5^2P excited states; ˜ 3-4 larger than the direct ionisation contribution predicted by CCC at ˜ 30-50 eV. This surprising result shows the importance of multi-electron processes in determining the ionisation cross sections of heavy alkali atoms.

  10. Cross sections for electron collisions with dimethyl ether

    NASA Astrophysics Data System (ADS)

    Sugohara, R. T.; Homem, M. G. P.; Iga, I.; de Souza, G. L. C.; Machado, L. E.; Ferraz, J. R.; dos Santos, A. S.; Brescansin, L. M.; Lucchese, R. R.; Lee, M. T.

    2013-08-01

    We report a joint theoretical-experimental investigation of electron collision with dimethyl ether (DME) in the low- and intermediate-energy ranges. Experimental absolute differential, integral, and momentum-transfer cross sections for elastic e--DME scattering are reported in the 100-1000 eV energy range. Our measurements were performed using a crossed electron-beam-molecular-beam geometry. The angular distribution of the scattered electrons was converted to absolute cross section using the relative flow technique. Theoretically, elastic differential, integral, and momentum-transfer cross sections, as well as the grand-total and total absorption cross sections for electron collision with DME are calculated in the 1-1000 eV energy range. A single-center-expansion technique combined with the Padé approximant method is used in our calculations. A comparison between the present experimental and theoretical data shows very good agreement. Moreover, comparison with theoretical and experimental data for e--ethanol (an isomer of DME) scattering shows interesting isomeric effects.

  11. Measurement of proton inelastic scattering cross sections on fluorine

    NASA Astrophysics Data System (ADS)

    Chiari, M.; Caciolli, A.; Calzolai, G.; Climent-Font, A.; Lucarelli, F.; Nava, S.

    2016-10-01

    Differential cross-sections for proton inelastic scattering on fluorine, 19F(p,p')19F, from the first five excited levels of 19F at 110, 197, 1346, 1459 and 1554 keV were measured for beam energies from 3 to 7 MeV at a scattering angle of 150° using a LiF thin target (50 μg/cm2) evaporated on a self-supporting C thin film (30 μg/cm2). Absolute differential cross-sections were calculated with a method not dependent on the absolute values of collected beam charge and detector solid angle. The validity of the measured inelastic scattering cross sections was then tested by successfully reproducing EBS spectra collected from a thick Teflon (CF2) target. As a practical application of these measured inelastic scattering cross sections in elastic backscattering spectroscopy (EBS), the feasibility of quantitative light element (C, N and O) analysis in aerosol particulate matter samples collected on Teflon by EBS measurements and spectra simulation is demonstrated.

  12. Vertically stabilized elongated cross-section tokamak

    DOEpatents

    Sheffield, George V.

    1977-01-01

    This invention provides a vertically stabilized, non-circular (minor) cross-section, toroidal plasma column characterized by an external separatrix. To this end, a specific poloidal coil means is added outside a toroidal plasma column containing an endless plasma current in a tokamak to produce a rectangular cross-section plasma column along the equilibrium axis of the plasma column. By elongating the spacing between the poloidal coil means the plasma cross-section is vertically elongated, while maintaining vertical stability, efficiently to increase the poloidal flux in linear proportion to the plasma cross-section height to achieve a much greater plasma volume than could be achieved with the heretofore known round cross-section plasma columns. Also, vertical stability is enhanced over an elliptical cross-section plasma column, and poloidal magnetic divertors are achieved.

  13. Normalization of experimental electron cross sections.

    NASA Astrophysics Data System (ADS)

    Avdonina, N.; Felfli, Z.; Msezane, A. Z.

    1997-10-01

    Absolute experimental electron-impact differential cross sections (DCSs) can be obtained through an extrapolation of the relative generalized oscillator strength (GOS) values at some given impact energy E to zero momentum transfer squared K^2, the optical oscillator strength (OOS) [1]. We propose to normalize the relative experimental DCS data to the corresponding OOS value by extrapolating the GOS to K^2 = 0 without involving the nonphysical region. This is possible only by simultaneously increasing E and decreasing K^2 so that K^2 = 0 corresponds to E = ∞. Thus is avoided a divergence of fracd(GOS)d(K^2) at K^2 = 0 [2]. Another advantage of our method is that, over a wide range of small K^2 values the contribution of higher order terms of the Born series to the GOS function is negligible, contrary to the constant E case in which even order K^2 terms are non-Born [2]. Thus first Born approximation can be used to normalize relative experimental DCSs to the OOS. This method is applicable to both the excitation and ionization of atomic and molecular targets by electron impact. The latter case generalizes the method of ref. [3]. ^*Supported by AFOSR, NSF and DoE Div. of Chemical Sciences, OBES. ^1 E. N. Lassettre et al., J. Chem. Phys \\underline50, (1829) ^2 W. M. Huo, J. Chem. Phys \\underline71, 1593 (1979) ^3 A. Saenz, W Weyrich and P. Froelich, J. Phys. B \\underline29, 97 (1996)

  14. Cross sections for ultra-low-energy electron scattering from atoms and molecules

    NASA Astrophysics Data System (ADS)

    Kitajima, M.; Shigemura, K.; Hosaka, K.; Odagiri, T.; Hoshino, M.; Tanaka, H.

    2016-12-01

    Absolute total cross sections for electron scattering from He, Ne, Ar, Kr and Xe at very low electron energies obtained using the technique employing the threshold-photoelectron source are presented. Comparison of the measured cross section for noble gas atoms with those of theoretical results are made.

  15. Cross Sections for Electron Collisions with Acetylene

    NASA Astrophysics Data System (ADS)

    Song, Mi-Young; Yoon, Jung-Sik; Cho, Hyuck; Karwasz, Grzegorz P.; Kokoouline, Viatcheslav; Nakamura, Yoshiharu; Tennyson, Jonathan

    2017-03-01

    Cross section data are compiled from the literature for electron collisions with the acetylene (HCCH) molecule. Cross sections are collected and reviewed for total scattering, elastic scattering, momentum transfer, excitations of rotational and vibrational states, dissociation, ionization, and dissociative attachment. The data derived from swarm experiments are also considered. For each of these processes, the recommended values of the cross sections are presented. The literature has been surveyed through early 2016.

  16. Cross Sections for Electron Collisions with Methane

    SciTech Connect

    Song, Mi-Young Yoon, Jung-Sik; Cho, Hyuck; Itikawa, Yukikazu; Karwasz, Grzegorz P.; Kokoouline, Viatcheslav; Nakamura, Yoshiharu; Tennyson, Jonathan

    2015-06-15

    Cross section data are compiled from the literature for electron collisions with methane (CH{sub 4}) molecules. Cross sections are collected and reviewed for total scattering, elastic scattering, momentum transfer, excitations of rotational and vibrational states, dissociation, ionization, and dissociative attachment. The data derived from swarm experiments are also considered. For each of these processes, the recommended values of the cross sections are presented. The literature has been surveyed through early 2014.

  17. Annular-Cross-Section CFE Chamber

    NASA Technical Reports Server (NTRS)

    Sharnez, Rizwan; Sammons, David W.

    1994-01-01

    Proposed continuous-flow-electrophoresis (CFE) chamber of annular cross section offers advantages over conventional CFE chamber, and wedge-cross-section chamber described in "Increasing Sensitivity in Continuous-Flow Electrophoresis" (MFS-26176). In comparison with wedge-shaped chamber, chamber of annular cross section virtually eliminates such wall effects as electro-osmosis and transverse gradients of velocity. Sensitivity enhanced by incorporating gradient maker and radial (collateral) flow.

  18. Annular-Cross-Section CFE Chamber

    NASA Technical Reports Server (NTRS)

    Sharnez, Rizwan; Sammons, David W.

    1994-01-01

    Proposed continuous-flow-electrophoresis (CFE) chamber of annular cross section offers advantages over conventional CFE chamber, and wedge-cross-section chamber described in "Increasing Sensitivity in Continuous-Flow Electrophoresis" (MFS-26176). In comparison with wedge-shaped chamber, chamber of annular cross section virtually eliminates such wall effects as electro-osmosis and transverse gradients of velocity. Sensitivity enhanced by incorporating gradient maker and radial (collateral) flow.

  19. Theoretical antideuteron-nucleus absorptive cross sections

    NASA Technical Reports Server (NTRS)

    Buck, W. W.; Norbury, J. W.; Townsend, L. W.; Wilson, J. W.

    1993-01-01

    Antideuteron-nucleus absorptive cross sections for intermediate to high energies are calculated using an ion-ion optical model. Good agreement with experiment (within 15 percent) is obtained in this same model for (bar p)-nucleus cross sections at laboratory energies up to 15 GeV. We describe a technique for estimating antinucleus-nucleus cross sections from NN data and suggest that further cosmic ray studies to search for antideuterons and other antinuclei be undertaken.

  20. Neutron capture cross section of 102Pd

    NASA Astrophysics Data System (ADS)

    Duncan, C. L.; Krane, K. S.

    2005-05-01

    The cross sections for radiative neutron capture by 102Pd have been deduced from a measurement of the γ rays emitted by 17.0-d 103Pd. The thermal cross section has been determined to be σ=1.82±0.20 b, and the effective resonance integral is I=23±4 b. We also report thermal and resonance capture cross sections for 108Pd and note possible inconsistencies with the presently accepted values of the 110Pd cross sections.

  1. Froissart bound on inelastic cross section without unknown constants

    NASA Astrophysics Data System (ADS)

    Martin, André; Roy, S. M.

    2015-04-01

    Assuming that axiomatic local field theory results hold for hadron scattering, André Martin and S. M. Roy recently obtained absolute bounds on the D wave below threshold for pion-pion scattering and thereby determined the scale of the logarithm in the Froissart bound on total cross sections in terms of pion mass only. Previously, Martin proved a rigorous upper bound on the inelastic cross-section σinel which is one-fourth of the corresponding upper bound on σtot, and Wu, Martin, Roy and Singh improved the bound by adding the constraint of a given σtot. Here we use unitarity and analyticity to determine, without any high-energy approximation, upper bounds on energy-averaged inelastic cross sections in terms of low-energy data in the crossed channel. These are Froissart-type bounds without any unknown coefficient or unknown scale factors and can be tested experimentally. Alternatively, their asymptotic forms, together with the Martin-Roy absolute bounds on pion-pion D waves below threshold, yield absolute bounds on energy-averaged inelastic cross sections. For example, for π0π0 scattering, defining σinel=σtot-(σπ0π0→π0π0+σπ0π0→π+π-) , we show that for c.m. energy √{s }→∞, σ¯ inel(s ,∞)≡s ∫s∞d s'σinel(s')/s'2≤(π /4 )(mπ)-2[ln (s /s1)+(1 /2 )ln ln (s /s1)+1 ]2 where 1 /s1=34 π √{2 π }mπ-2 . This bound is asymptotically one-fourth of the corresponding Martin-Roy bound on the total cross section, and the scale factor s1 is one-fourth of the scale factor in the total cross section bound. The average over the interval (s,2s) of the inelastic π0π0 cross section has a bound of the same form with 1 /s1 replaced by 1 /s2=2 /s1.

  2. Photoionization of atoms and molecules. [of hydrogen, helium, and xenon

    NASA Technical Reports Server (NTRS)

    Samson, J. A. R.

    1976-01-01

    A literature review on the present state of knowledge in photoionization is presented. Various experimental techniques that have been developed to study photoionization, such as fluorescence and photoelectron spectroscopy, mass spectroscopy, are examined. Various atoms and molecules were chosen to illustrate these techniques, specifically helium and xenon atoms and hydrogen molecules. Specialized photoionization such as in positive and negative ions, excited states, and free radicals is also treated. Absorption cross sections and ionization potentials are also discussed.

  3. Photoionization Dynamics of Small Molecules

    SciTech Connect

    Dehmer, Joseph L.; Dill, Dan; Parr, Albert C.

    1985-01-01

    The last decade has witnessed remarkable progress in characterizing dynamical aspects of the molecular photoionization process. The general challenge is to gain physical insight into those processes occuring during photo excitation and eventual escape of the photoelectron through the anisotropic molecular field, in terms of various observables such as photoionization cross-sections and branching ratios, photoelectron angular distributions and even newer probes mentioned below. Much of the progress in this field has mirrored earlier work in atomic photoionization dynamics where many key ideas were developed (e.g., channel interaction, quantum defect analysis, potential barrier phenomena and experimental techniques). However, additional concepts and techniques were required to deal with the strictly molecular aspects of the problem, particularly the anisotropy of the multicenter molecular field and the interaction among rovibronic modes.

  4. Laboratory study of K-shell photoionization of oxygen and oxygen hydrides ions

    NASA Astrophysics Data System (ADS)

    Bizau, Jean-Marc

    2016-05-01

    The interpretation of the spectra sent by satellites required the knowledge of many atomic data, including photoionization cross sections or energy and oscillator strength of bound-bound transitions for many ions, over a broad photon energy range going from infra-red to x-rays. These data are mainly provided by theoretical results using state-of-the-art methods like R-matrix. Recently, discrepancies have been observed between the calculated energy of the Kα transitions in atomic oxygen and its ions and those determined from the satellites observations. The results of the experimental studies of K-shell photoionization of oxygen ions performed at the French synchrotron radiation center SOLEIL will be presented. A merged-beam setup installed on the PLEIADES beam line allows for the determination of absolute photoionization cross sections and transitions energy on singly- and multiply-charged ions in the 10-1000 eV photon energy range. The first results obtained with this setup on oxygen hydrides will be also presented.

  5. Photoionization Efficiencies of Five Polycyclic Aromatic Hydrocarbons

    DOE PAGES

    Johansson, K. Olof; Campbell, Matthew F.; Elvati, Paolo; ...

    2017-05-18

    We have measured photoionization-efficiency curves for pyrene, fluoranthene, chrysene, perylene, and coronene in the photon energy range of 7.5-10.2 eV and derived their photoionization cross-section curves in this energy range. All measurements were performed using tunable vacuum ultraviolet (VUV) radiation generated at the Advanced Light Source synchrotron at Lawrence Berkeley National Laboratory. The VUV radiation was used for photoionization, and detection was performed using a time-of-flight mass spectrometer. We measured the photoionization efficiency of 2,5-dimethylfuran simultaneously with those of pyrene, fluoranthene, chrysene, perylene, and coronene to obtain references of the photon flux during each measurement from the known photoionization cross-sectionmore » curve of 2,5- dimethylfuran.« less

  6. Neutrino flux predictions for cross section measurements

    SciTech Connect

    Hartz, Mark

    2015-05-15

    Experiments that measure neutrino interaction cross sections using accelerator neutrino sources require a prediction of the neutrino flux to extract the interaction cross section from the measured neutrino interaction rate. This article summarizes methods of estimating the neutrino flux using in-situ and ex-situ measurements. The application of these methods by current and recent experiments is discussed.

  7. Neutrino Cross Sections at Solar Energies

    NASA Astrophysics Data System (ADS)

    Strigari, Louis

    2017-01-01

    I will review neutrino nucleus cross section measurements and uncertainties for energies applicable to solar neutrinos. I will discuss how these cross sections are important for interpreting solar neutrino experimental data, and highlight the most important neutrino-nucleus interactions that will be relevant for forthcoming dark matter direct detection experiments. NSF PHY-1522717.

  8. The absolute absorption cross section of crystalline αg and βg HNO33H2O (NAT) and HNO32H2O (NAD) in the range 180 - 200 K in the mid-IR (4000 to 600 cm-1)

    NASA Astrophysics Data System (ADS)

    Rossi, Michel J.; Iannarelli, Riccardo

    2014-05-01

    Heterogeneous processing in the polar atmosphere requires the presence of polar stratospheric cloud particles (PSC's) that are the seat of interfacial chlorine and NOx chemistry. A subgroup of PSC's, namely PSC Ia, are known to consist of hydrates of nitric acid, mostly nitric acid trihydrate (NAT) as two polymorphs, α- and β-HNO33H2O occurring in the range 185 to 200 K under prevailing stratospheric partial pressure conditions of 10 ppb HNO3 or so. Despite the fact that reference IR spectra in the mid-IR range have been obtained some time ago (Ritzhaupt and Devlin (1991), Koehler et al. (1992)), no absolute absorption cross section of these important ice particles exist to date except a study of its refractive indices (Middlebrook et al. (1994), Berland et al. (1994)). Knowledge of optical cross sections would enable remote sensing of PSC's in the IR region using satellite and/or LIDAR platforms. We have embarked on a multidiagnostic research program aiming at studying the kinetics, thermodynamics and spectroscopy of PSC's using a stirred flow reactor equipped with FTIR absorption spectroscopy in transmission. The gas phase was monitored using electron-impact residual gas mass spectroscopy together with pulsed and steady-state gas admission and thorough characterization of the adsorption of HNO3, H2O and HCl onto the stainless-steel vessel walls under mass balance conditions using measured Langmuir adsorption isotherms. We have grown α- and β-NAT by doping thin (1 μm thick) ice films with metered amounts of HNO3. According to known phase diagrams we have obtained mixtures of pure ice with NAT whose IR spectrum was obtained after spectral subtraction of the pure ice phase. The concentration of HNO3 deposited on the ice film was determined by measuring the inflow and taking into account adsorption of HNO3 on the reactor walls as well as effusive loss out the reactor. We also independently checked the H2O concentration of α-NAT from the decrease of the pure H2O

  9. Photon scattering cross sections of H2 and He measured with synchrotron radiation

    NASA Technical Reports Server (NTRS)

    Ice, G. E.

    1977-01-01

    Total (elastic + inelastic) differential photon scattering cross sections have been measured for H2 gas and He, using an X-ray beam. Absolute measured cross sections agree with theory within the probable errors. Relative cross sections (normalized to theory at large S) agree to better than one percent with theoretical values calculated from wave functions that include the effect of electron-electron Coulomb correlation, but the data deviate significantly from theoretical independent-particle (e.g., Hartree-Fock) results. The ratios of measured absolute He cross sections to those of H2, at any given S, also agree to better than one percent with theoretical He-to-H2 cross-section ratios computed from correlated wave functions. It appears that photon scattering constitutes a very promising tool for probing electron correlation in light atoms and molecules.

  10. Energy and angle differential cross sections for the electron-impact double ionization of helium

    SciTech Connect

    Colgan, James P; Pindzola, M S; Robicheaux, F

    2008-01-01

    Energy and angle differential cross sections for the electron-impact double ionization of helium are calculated using a non-perturbative time-dependent close-coupling method. Collision probabilities are found by projection of a time evolved nine dimensional coordinate space wave function onto fully antisymmetric products of spatial and spin functions representing three outgoing Coulomb waves. At an incident energy of 106 eV, we present double energy differential cross sections and pentuple energy and angle differential cross sections. The pentuple energy and angle differential cross sections are found to be in relative agreement with the shapes observed in recent (e,3e) reaction microscope experiments. Integration of the differential cross sections over all energies and angles yields a total ionization cross section that is also in reasonable agreement with absolute crossed-beams experiments.

  11. Double K-shell photoionization and universal scaling laws

    NASA Astrophysics Data System (ADS)

    Hoszowska, J.; Kheifets, A. K.; Dousse, J.-Cl; Berset, M.; Bray, I.; Cao, W.; Fennane, K.; Kayser, Y.; Kavčič, M.; Szlachetko, J.; Szlachetko, M.

    2009-11-01

    The photon energy dependence of the double K-shell ionization cross sections for light atoms and He-like ions is reported. The K-shell double photoionization DPI cross-sections for hollow atom production are compared to those of the corresponding He-like counterparts. The relative contribution of the initial-state correlations and final-state electron-electron interactions to the K-shell DPI is addressed. A semiempirical universal scaling of the double photoionization cross sections with the effective nuclear charge for neutral atoms in the range 2 <= Z <= 47 is established.

  12. Excitation and Charge Exchange Phenomena in Astronomical Objects: Measurement of Cross Sections and Lifetimes

    NASA Technical Reports Server (NTRS)

    Chutjian, Ara; Smith, S.; Lozano, J.; Cadez, I.; Greewnood, J.; Mawhovter, R.; Williams, I.; Niimura, M.

    2003-01-01

    This document addresses extreme ultraviolet radiation and X-ray emissions from comets, planets and heliospheric gases focusing on the measurement of charge-exchange cross sections and radiative lifetimes. Highly-charged heavy ions present in the solar wind, and their abundance relative to the total oxygen-ion abundance are detailed. The plan for the Jet Propulsion Laboratory high-charge ion facility is outlined detailing its ability to measure absolute collisional excitation cross sections, absolute charge-exchange cross sections, lifetimes of metastable ion levels, and X-ray emission spectra following charge changes.

  13. Excitation and Charge Exchange Phenomena in Astronomical Objects: Measurement of Cross Sections and Lifetimes

    NASA Technical Reports Server (NTRS)

    Chutjian, Ara; Smith, S.; Lozano, J.; Cadez, I.; Greewnood, J.; Mawhovter, R.; Williams, I.; Niimura, M.

    2003-01-01

    This document addresses extreme ultraviolet radiation and X-ray emissions from comets, planets and heliospheric gases focusing on the measurement of charge-exchange cross sections and radiative lifetimes. Highly-charged heavy ions present in the solar wind, and their abundance relative to the total oxygen-ion abundance are detailed. The plan for the Jet Propulsion Laboratory high-charge ion facility is outlined detailing its ability to measure absolute collisional excitation cross sections, absolute charge-exchange cross sections, lifetimes of metastable ion levels, and X-ray emission spectra following charge changes.

  14. Spectrally resolved fluorescence cross sections of BG and BT with a 266-nm pump wavelength

    NASA Astrophysics Data System (ADS)

    Atkins, Joshua; Thomas, Michael E.; Joseph, Richard I.

    2007-04-01

    The spectrally resolved absolute fluorescence cross sections of Bacillus globigii (BG) and Bacillus thuringiensis (BT) were measured with a 266nm Nd:YAG laser source. The aerosol samples were prepared in dilute aqueous suspensions for measurement and the absolute cross section was found by use of the Raman scattering line from water. Integrated cross sections for BT and BG were found to be 1.1864 × 10 -12 cm2(spore sr) and 3.251 × 10 -13 cm2/ (spore sr) respectively.

  15. Direct double photoionization of the valence shell of Be

    SciTech Connect

    Citrini, F.; Malegat, L.; Selles, P.; Kazansky, A.K.

    2003-04-01

    The hyperspherical R-matrix method with semiclassical outgoing waves is used to study the direct double photoionization (DPI) of the valence shell of the lightest alkaline earth-metal Be. The absolute fully integrated, singly, doubly, and triply differential cross sections obtained are compared with the single set of measurements available and with recent calculations based on the convergent close coupling and time-dependent close coupling methods. The level of agreement between all these data is very encouraging. A comparison is also made between the DPI of He and the direct DPI of the valence shell of Be. It confirms that the electron-electron correlations are stronger in the valence 2s shell of Be than in the 1s shell of He, thus contributing to a desirable clarification.

  16. Partial cross sections of helium satellites at medium photon energies

    SciTech Connect

    Wehlitz, R.; Sellin, I.A.; Hemmers, O.

    1997-04-01

    Still of current interest is the important role of single ionization with excitation compared to single ionization alone. The coupling between the electrons and the incoming photon is a single-particle operator. Thus, an excitation in addition to an ionization, leading to a so-called satellite line in a photoelectron spectrum, is entirely due to electron-electron interaction and probes the electron correlation in the ground and final state. Therefore the authors have undertaken the study of the intensity of helium satellites He{sup +}nl (n = 2 - 6) relative to the main photoline (n = 1) as a function of photon energy at photon energies well above threshold up to 900 eV. From these results they could calculate the partial cross-sections of the helium satellites. In order to test the consistency of their satellite-to-1s ratios with published double-to-single photoionization ratios, the authors calculated the double-to-single photoionization ratio from their measured ratios using the theoretical energy-distribution curves of Chang and Poe and Le Rouzo and Dal Cappello which proved to be valid for photon energies below 120 eV. These calculated double-to-single ionization ratios agree fairly well with recent ion measurements. In the lower photon energy range the authors ratios agree better with the ratios of Doerner et al. while for higher photon energies the agreement is better with the values of Levin et al.

  17. Photodetachment cross-section evaluation using asymptotic considerations

    NASA Astrophysics Data System (ADS)

    Babilotte, Philippe; Vandevraye, Mickael

    2017-06-01

    Mathematical calculations are given concerning the evaluation of the negative ions photodetachment cross-section σ , into a so-called saturation regime. The interaction between a negative ion particle beam and a laser beam is examined under theoretical aspects. A quantitative criterion S is proposed to define the saturation threshold between the linear and the saturated domains, which are both present in this saturation regime. The asymptotic behaviours extracted at the low and high energy limits are used to determine this threshold quantitative criterion S and to evaluate also the photodetachment cross-section σ . The case of a symmetric gaussian photodetachment laser beam shape is examined according to the proposed formalism, which can be used either for the photo-detachment or photo-ionization processes, and could be potentially used into technological solutions for negative ion neutralisation processes (such as neutral beam injector) in the future fusion energy devices. Estimations onto the errors related to the use of this methodology are given.

  18. Nucleon-Nucleon Total Cross Section

    NASA Technical Reports Server (NTRS)

    Norbury, John W.

    2008-01-01

    The total proton-proton and neutron-proton cross sections currently used in the transport code HZETRN show significant disagreement with experiment in the GeV and EeV energy ranges. The GeV range is near the region of maximum cosmic ray intensity. It is therefore important to correct these cross sections, so that predictions of space radiation environments will be accurate. Parameterizations of nucleon-nucleon total cross sections are developed which are accurate over the entire energy range of the cosmic ray spectrum.

  19. Cross-sectional anatomy for computed tomography

    SciTech Connect

    Farkas, M.L.

    1988-01-01

    This self-study guide recognizes that evaluation and interpretation of CT-images demands a firm understanding of both cross-sectional anatomy and the principles of computed tomography. The objectives of this book are: to discuss the basic principles of CT, to stress the importance of cross-sectional anatomy to CT through study of selected cardinal transverse sections of head, neck, and trunk, to explain orientation and interpretation of CT-images with the aid of corresponding cross-sectional preparations.

  20. Ultrahigh-energy photonuclear cross sections

    SciTech Connect

    Gandhi, R.; Sarcevic, I.; Burrows, A. ); Durand, L.; Pi, H. )

    1990-07-01

    We present results of calculations of the total inelastic photon-air cross sections at ultrahigh energies (up to 10{sup 8} GeV in the laboratory) of relevance to on-going cosmic-ray experiments. The calculations take into account the high-energy QCD structure of the photon and are performed for a variety of photon and proton structure functions. The total inelastic photon-air cross section is obtained from the photon-proton jet cross section via an eikonalization procedure using a QCD-based diffractive model. The results are discussed in the context of the apparent excess muon content of air showers associated with point sources.

  1. Cross Section Evaluations for Arsenic Isotopes

    SciTech Connect

    Pruet, J; McNabb, D P; Ormand, W E

    2005-03-10

    The authors present an evaluation of cross sections describing reactions with neutrons incident on the arsenic isotopes with mass numbers 75 and 74. Particular attention is paid to (n,2n) reactions. The evaluation for {sup 75}As, the only stable As isotope, is guided largely by experimental data. Evaluation for {sup 74}As is made through calculations with the EMPIRE statistical-model reaction code. Cross sections describing the production and destruction of the 26.8 ns isomer in {sup 74}As are explicitly considered. Uncertainties and covariances in some evaluated cross sections are also estimated.

  2. Neutron Capture Cross Section of 239Pu

    NASA Astrophysics Data System (ADS)

    Mosby, S.; Arnold, C.; Bredeweg, T. A.; Chyzh, A.; Couture, A.; Henderson, R.; Jandel, M.; Kwan, E.; O'Donnell, J. M.; Rusev, G.; Ullmann, J. L.; Wu, C. Y.

    2014-05-01

    The Detector for Advanced Neutron Capture Experiments (DANCE) has been used to measure the 239Pu(n,γ) cross section from 10 eV to the keV region. Three experimental run conditions were used to characterize the prompt fission γ-ray spectrum across the entire energy regime, measure the cross section in the resolved resonance region, and obtain necessary count rate well into the keV region. The preliminary cross sections are in good agreement with current evaluations from 10 eV to 80 keV.

  3. Measurement of the Absolute Raman Cross Sections of Diethyl Phthalate, Dimethyl Phthalate, Ethyl Cinnamate, Propylene Carbonate, Tripropyl Phosphate, 1,3-Cyclohexanedione, 3’-Aminoacetophenone, 3’-Hydroxyacetophenone, Diethyl Acetamidomalonate, Isovanillin, Lactide, Meldrum’s Acid, p-Tolyl Sulfoxide, and Vanillin

    DTIC Science & Technology

    2013-09-13

    Propylene Carbonate , Tripropyl Phosphate, 1,3-Cyclohexanedione, 3’-Aminoacetophenone, 3’-Hydroxyacetophenone, Diethyl Acetamidomalonate, Isovanillin...Cross Sections of Diethyl Phthalate, Dimethyl Phthalate, Ethyl Cinnamate, Propylene Carbonate , Tripropyl Phosphate, 1,3-Cyclohexanedione, 3...been determined for the Raman cross section σR of neat Diethyl phthalate (DEP), dimethyl phthalate (DMP), ethyl cinnamate (EC), propylene carbonate

  4. A coupled-cluster study of photodetachment cross sections of closed-shell anions.

    PubMed

    Cukras, Janusz; Decleva, Piero; Coriani, Sonia

    2014-11-07

    We investigate the performance of Stieltjes Imaging applied to Lanczos pseudo-spectra generated at the coupled cluster singles and doubles, coupled cluster singles and approximate iterative doubles and coupled cluster singles levels of theory in modeling the photodetachment cross sections of the closed shell anions H(-), Li(-), Na(-), F(-), Cl(-), and OH(-). The accurate description of double excitations is found to play a much more important role than in the case of photoionization of neutral species.

  5. Photoionization of P+: Experiment and theory

    NASA Astrophysics Data System (ADS)

    Nahar, S. N.; Hernández, E. M.; Hernández, L.; Antillón, A.; Morales-Mori, A.; González, O.; Covington, A. M.; Chartkunchand, K. C.; Hanstorp, D.; Juárez, A. M.; Hinojosa, G.

    2017-01-01

    An experimental and theoretical study of the single photoionization cross section of the P+ cation of phosphorus is presented. Photoionization (PI) cross sections are instrumental for the determination of abundances in the interstellar medium. The experiment was performed by merging an ion beam with a photon beam. The photon beam was nearly monochromatic and had an energy resolution of 24 meV. Calculations were carried out using the Breit-Pauli R-matrix method. The combined study was developed in the photon energy interval from 18 eV (68.9 nm) to 50 eV (24.8 nm). Comparison between the measured and the calculated cross section shows good agreement in general and identifies features of the process and existence of states in the experimental beam. The present results should provide for more accurate modeling of P+.

  6. Energy dependence of fusion cross sections

    SciTech Connect

    Bang, J.M.; Ferreira, L.S.; Maglione, E.; Hansteen, J.M.

    1996-01-01

    Observed enhancements of fusion cross sections at low energies are explained as caused by an underestimate of beam energy due to an overestimate of the stopping energy loss. {copyright} {ital 1996 The American Physical Society.}

  7. A nuclear cross section data handbook

    SciTech Connect

    Fisher, H.O.M.

    1989-12-01

    Isotopic information, reaction data, data availability, heating numbers, and evaluation information are given for 129 neutron cross-section evaluations, which are the source of the default cross sections for the Monte Carlo code MCNP. Additionally, pie diagrams for each nuclide displaying the percent contribution of a given reaction to the total cross section are given at 14 MeV, 1 MeV, and thermal energy. Other information about the evaluations and their availability in continuous-energy, discrete-reaction, and multigroup forms is provided. The evaluations come from ENDF/B-V, ENDL85, and the Los Alamos Applied Nuclear Science Group T-2. Graphs of all neutron and photon production cross-section reactions for these nuclides have been categorized and plotted. 21 refs., 5 tabs.

  8. Bibliography of photoabsorption cross-section data

    NASA Technical Reports Server (NTRS)

    Hudson, R. D.; Kieffer, L. J.

    1970-01-01

    This bibliography contains only references which report a measured or calculated photoabsorption cross section (relative or normalized) in regions of continuous absorption. The bibliography is current as of January 1, 1970.

  9. The radar cross section of dielectric disks

    NASA Technical Reports Server (NTRS)

    Levine, D. M.

    1982-01-01

    A solution is presented for the backscatter (nonstatic) radar cross section of dielectric disks of arbitrary shape, thickness and dielectric constant. The result is obtained by employing a Kirchhoff type approximation to obtain the fields inside the disk. The internal fields induce polarization and conduction currents from which the scattered fields and the radar cross section can be computed. The solution for the radar cross section obtained in this manner is shown to agree with known results in the special cases of normal incidence, thin disks and perfect conductivity. The solution can also be written as a product of the reflection coefficient of an identically oriented slab times the physical optics solution for the backscatter cross section of a perfectly conducting disk of the same shape. This result follows directly from the Kirchhoff type approximation without additional assumptions.

  10. Dijet cross sections in photoproduction at HERA

    NASA Astrophysics Data System (ADS)

    ZEUS Collaboration; Breitweg, J.; et al.

    Dijet cross sections are presented using photoproduction data obtained with the ZEUS detector during 1994. These measurements represent an extension of previous results, as the higher statistics allow cross sections to be measured at higher jet transverse energy ( ETjet). Jets are identified in the hadronic final state using three different algorithms, and the cross sections compared to complete next-to-leading order QCD calculations. Agreement with these calculations is seen for the pseudorapidity dependence of the direct photon events with ETjet > 6 GeV and of the resolved photon events with ETjet > 11 GeV. Calculated cross sections for resolved photon processes with 6 GeV < ETjet < 11 GeV lie below the data.

  11. Capture cross sections on unstable nuclei

    NASA Astrophysics Data System (ADS)

    Tonchev, A. P.; Escher, J. E.; Scielzo, N.; Bedrossian, P.; Ilieva, R. S.; Humby, P.; Cooper, N.; Goddard, P. M.; Werner, V.; Tornow, W.; Rusev, G.; Kelley, J. H.; Pietralla, N.; Scheck, M.; Savran, D.; Löher, B.; Yates, S. W.; Crider, B. P.; Peters, E. E.; Tsoneva, N.; Goriely, S.

    2017-09-01

    Accurate neutron-capture cross sections on unstable nuclei near the line of beta stability are crucial for understanding the s-process nucleosynthesis. However, neutron-capture cross sections for short-lived radionuclides are difficult to measure due to the fact that the measurements require both highly radioactive samples and intense neutron sources. Essential ingredients for describing the γ decays following neutron capture are the γ-ray strength function and level densities. We will compare different indirect approaches for obtaining the most relevant observables that can constrain Hauser-Feshbach statistical-model calculations of capture cross sections. Specifically, we will consider photon scattering using monoenergetic and 100% linearly polarized photon beams. Challenges that exist on the path to obtaining neutron-capture cross sections for reactions on isotopes near and far from stability will be discussed.

  12. Benchmark cross sections for bottom quark production

    SciTech Connect

    Berger, E.L.

    1988-01-07

    A summary is presented of theoretical expectations for the total cross sections for bottom quark production, for longitudinal and transverse momentum distributions, and for b, /bar b/ momentum correlations at Fermilab fixed target and collider energies.

  13. MODELING AND FISSION CROSS SECTIONS FOR AMERICIUM.

    SciTech Connect

    ROCHMAN, D.; HERMAN, M.; OBLOZINSKY, P.

    2005-05-01

    This is the final report of the work performed under the LANL contract on the modeling and fission cross section for americium isotopes (May 2004-June 2005). The purpose of the contract was to provide fission cross sections for americium isotopes with the nuclear reaction model code EMPIRE 2.19. The following work was performed: (1) Fission calculations capability suitable for americium was implemented to the EMPIRE-2.19 code. (2) Calculations of neutron-induced fission cross sections for {sup 239}Am to {sup 244g}Am were performed with EMPIRE-2.19 for energies up to 20 MeV. For the neutron-induced reaction of {sup 240}Am, fission cross sections were predicted and uncertainties were assessed. (3) Set of fission barrier heights for each americium isotopes was chosen so that the new calculations fit the experimental data and follow the systematics found in the literature.

  14. The radar cross section of dielectric disks

    NASA Technical Reports Server (NTRS)

    Le Vine, D. M.

    1984-01-01

    A solution is presented for the backscatter (monostatic) radar cross section of dielectric disks of arbitrary shape, thickness, and dielectric constant. The result is obtained by employing a Kirchhoff-type approximation to obtain the fields inside the disk. The internal fields induce polarization and conduction currents from which the scattered fields and the radar cross section can be computed. The solution for the radar cross section obtained in this manner will be shown to agree with known results in the special cases of normal incidence, thin disks, and perfect conductivity. It will also be shown that the solution can be written as a product of the reflection coefficient of an identically oriented slab times the physical optics solution for the backscatter cross section of a perfectly conducting disk of the same shape. This result follows directly from the Kirchhoff-type approximation without additional assumptions.

  15. Ultraviolet absorption cross sections of hydrogen peroxide

    NASA Technical Reports Server (NTRS)

    Lin, C. L.; Rohatgi, N. K.; Demore, W. B.

    1978-01-01

    Absorption cross-sections of hydrogen peroxide vapor and of neutral aqueous solutions of hydrogen peroxide were measured in the wavelength range from 195 to 350 nm at 296 K. The spectrophotometric procedure is described, and the reported cross-sections are compared with values obtained by other researchers. Photodissociation coefficients of atmospheric H2O2 were calculated for direct absorption of unscattered solar radiation, and the vertical distributions of these coefficients are shown for various solar zenith angles.

  16. High precision neutron inelastic cross section measurements

    NASA Astrophysics Data System (ADS)

    Olacel, A.; Belloni, F.; Borcea, C.; Boromiza, M.; Dessagne, Ph.; Henning, G.; Kerveno, M.; Negret, A.; Nyman, M.; Pirovano, E.; Plompen, A.

    2017-06-01

    High precision neutron inelastic scattering cross section data are very important for the development of the new generation of nuclear reactors (Gen IV). Our experiments, performed using the GELINA neutron source and the GAINS spectrometer of the European Commission Joint Research Center, Geel, produce highly reliable and precise cross section data. We will present the details of the setup and the data analysis technique allowing production of such unique results, and we will show examples of two experimental results.

  17. Reaction cross sections of unstable nuclei

    SciTech Connect

    Ozawa, Akira

    2006-11-02

    Experimental studies on reaction cross sections are reviewed. The recent developments of radioactive nuclear beams have enabled us to measure reaction cross-sections for unstable nuclei. Using Glauber-model analysis, effective nuclear matter density distributions of unstable nuclei can be studied. Recent measurements in RIBLL at IMP and RIPS at RIKEN are introduced. The effective matter density distributions for 14-18C are also mentioned.

  18. Shuttle orbiter radar cross-sectional analysis

    NASA Technical Reports Server (NTRS)

    Cooper, D. W.; James, R.

    1979-01-01

    Theoretical and model simulation studies on signal to noise levels and shuttle radar cross section are described. Pre-mission system calibrations, system configuration, and postmission system calibration of the tracking radars are described. Conversion of target range, azimuth, and elevation into radar centered east north vertical position coordinates are evaluated. The location of the impinging rf energy with respect to the target vehicles body axis triad is calculated. Cross section correlation between the two radars is presented.

  19. Selective detection of isomers with photoionization mass spectrometry for studies of hydrocarbon flame chemistry

    NASA Astrophysics Data System (ADS)

    Cool, Terrill A.; Nakajima, Koichi; Mostefaoui, Toufik A.; Qi, Fei; McIlroy, Andrew; Westmoreland, Phillip R.; Law, Matthew E.; Poisson, Lionel; Peterka, Darcy S.; Ahmed, Musahid

    2003-10-01

    We report the first use of synchrotron radiation, continuously tunable from 8 to 15 eV, for flame-sampling photoionization mass spectrometry (PIMS). Synchrotron radiation offers important advantages over the use of pulsed vacuum ultraviolet lasers for PIMS; these include superior signal-to-noise, soft ionization, and access to photon energies outside the limited tuning ranges of current VUV laser sources. Near-threshold photoionization efficiency measurements were used to determine the absolute concentrations of the allene and propyne isomers of C3H4 in low-pressure laminar ethylene-oxygen and benzene-oxygen flames. Similar measurements of the isomeric composition of C2H4O species in a fuel-rich ethylene-oxygen flame revealed the presence of substantial concentrations of ethenol (vinyl alcohol) and acetaldehyde. Ethenol has not been previously detected in hydrocarbon flames. Absolute photoionization cross sections were measured for ethylene, allene, propyne, and acetaldehyde, using propene as a calibration standard. PIE curves are presented for several additional reaction intermediates prominent in hydrocarbon flames.

  20. Dissociative and double photoionization of CO2 from threshold to 90 A

    NASA Technical Reports Server (NTRS)

    Masuoka, T.; Samson, J. A. R.

    1979-01-01

    The molecular photoionization, dissociative photoionization and double photoionization cross sections for CO2 were measured from their onsets down to 90 A by using various combinations of mass spectrometers (a coincidence time-of-flight mass spectrometer and a magnetic mass spectrometer) and light sources (synchrotron radiation, and glow and spark discharge). It is concluded that the one broad peak and the three shoulders in the total adsorption cross section curve between 640 and 90 A are caused completely by dissociative ionization processes. Several peaks observed in the cross section curve for the total fragmentation CO(+)3, O(+) and C(+) are compared with those in the photoelectron spectrum reported for CO2.

  1. Reduction Methods for Total Reaction Cross Sections

    NASA Astrophysics Data System (ADS)

    Gomes, P. R. S.; Mendes Junior, D. R.; Canto, L. F.; Lubian, J.; de Faria, P. N.

    2016-03-01

    The most frequently used methods to reduce fusion and total reaction excitation functions were investigated in a very recent paper Canto et al. (Phys Rev C 92:014626, 2015). These methods are widely used to eliminate the influence of masses and charges in comparisons of cross sections for weakly bound and tightly bound systems. This study reached two main conclusions. The first is that the fusion function method is the most successful procedure to reduce fusion cross sections. Applying this method to theoretical cross sections of single channel calculations, one obtains a system independent curve (the fusion function), that can be used as a benchmark to fusion data. The second conclusion was that none of the reduction methods available in the literature is able to provide a universal curve for total reaction cross sections. The reduced single channel cross sections keep a strong dependence of the atomic and mass numbers of the collision partners, except for systems in the same mass range. In the present work we pursue this problem further, applying the reduction methods to systems within a limited mass range. We show that, under these circumstances, the reduction of reaction data may be very useful.

  2. Undergraduate Measurements of Neutron Cross Sections

    NASA Astrophysics Data System (ADS)

    Hicks, S. F.; Vanhoy, J. R.; French, A. J.; Santonil, Z. C.; Crider, B. P.; Peters, E. E.; McEllistrem, M. T.; Prados-Estévez, F. M.; Ross, T. J.; Yates, S. W.

    Undergraduate students at the University of Dallas have investigated basic properties of nuclei through γ-ray and neutron spectroscopy following neutron scattering. The former has been used primarily for nuclear structure investigations, while the latter has been used to measure neutron scattering cross sections important for fission reactor applications. A series of (n,n') and (n,n'γ) measurements have been made on 54Fe and 56Fe to determine neutron cross sections for scattering to excited levels in these nuclei. The former provides the cross sections directly and the latter are used to deduce inelastic neutron scattering cross sections by measuring the γ-ray production cross sections to states not easily resolved in neutron spectroscopy. All measurements have been completed at the University of Kentucky Accelerator Laboratory using a 7-MV Model CN Van de Graaff accelerator, along with the neutron production and neutron and γ-ray detection systems located there. Students participate in accelerator operation, experimental setup, data acquisition, and data analyses. An overview of the research program and student contributions is presented.

  3. Absorption cross sections of stratospheric molecules

    NASA Technical Reports Server (NTRS)

    Hudson, R. D.

    1974-01-01

    Two classes of molecular species must be considered in a calculation of photochemical rates in the stratosphere. The first class consists of molecular oxygen and ozone, while the second class contains the remainder of the minor constituents. If accurate values of the transmitted fluxes are required at large optical depths, the cross sections for molecular oxygen and ozone must be known to within a few per cent at least. On the other hand, the photochemical rates for the minor species are given simply by the relevant cross sections. A review of published cross sections is presented, giving attention to molecular oxygen, ozone, nitric oxide, nitrogen dioxide, nitrous oxide, nitric acid, ammonia, water vapor, hydrogen peroxide, carbon monoxide, carbon dioxide, and sulfur dioxide.

  4. The cross section for double Compton scattering

    NASA Technical Reports Server (NTRS)

    Gould, R. J.

    1984-01-01

    Employing elementary methods in nonrelativistic quantum electrodynamics, the cross section for gamma sub 0 + e yields e + gamma + gamma is computed for arbitrary energy in the spectrum of the outgoing photons. The final result is given, differential in the energy of one of these photons, for the case where the incident photon is unpolarized and has energy E sub 0 much less than mc-squared, a polarization sum and angular integration being performed for the final-state photons. The cross section has a simple algebraic form resulting from contributions from the sum of squared direct and exchange amplitudes; interference terms from these amplitudes do not contribute to the angular-integrated cross section.

  5. Prospects for Precision Neutrino Cross Section Measurements

    SciTech Connect

    Harris, Deborah A.

    2016-01-28

    The need for precision cross section measurements is more urgent now than ever before, given the central role neutrino oscillation measurements play in the field of particle physics. The definition of precision is something worth considering, however. In order to build the best model for an oscillation experiment, cross section measurements should span a broad range of energies, neutrino interaction channels, and target nuclei. Precision might better be defined not in the final uncertainty associated with any one measurement but rather with the breadth of measurements that are available to constrain models. Current experience shows that models are better constrained by 10 measurements across different processes and energies with 10% uncertainties than by one measurement of one process on one nucleus with a 1% uncertainty. This article describes the current status of and future prospects for the field of precision cross section measurements considering the metric of how many processes, energies, and nuclei have been studied.

  6. Algorithmic analysis of quantum radar cross sections

    NASA Astrophysics Data System (ADS)

    Lanzagorta, Marco; Venegas-Andraca, Salvador

    2015-05-01

    Sidelobe structures on classical radar cross section graphs are a consequence of discontinuities in the surface currents. In contrast, quantum radar theory states that sidelobe structures on quantum radar cross section graphs are due to quantum interference. Moreover, it is conjectured that quantum sidelobe structures may be used to detect targets oriented off the specular direction. Because of the high data bandwidth expected from quantum radar, it may be necessary to use sophisticated quantum signal analysis algorithms to determine the presence of stealth targets through the sidelobe structures. In this paper we introduce three potential quantum algorithmic techniques to compute classical and quantum radar cross sections. It is our purpose to develop a computer science-oriented tool for further physical analysis of quantum radar models as well as applications of quantum radar technology in various fields.

  7. Top differential cross section measurements (Tevatron)

    SciTech Connect

    Jung, Andreas W.

    2012-01-01

    Differential cross sections in the top quark sector measured at the Fermilab Tevatron collider are presented. CDF used 2.7 fb{sup -1} of data and measured the differential cross section as a function of the invariant mass of the t{bar t} system. The measurement shows good agreement with the standard model and furthermore is used to derive limits on the ratio {kappa}/M{sub Pl} for gravitons which decay to top quarks in the Randall-Sundrum model. D0 used 1.0 fb{sup -1} of data to measure the differential cross section as a function of the transverse momentum of the top-quark. The measurement shows a good agreement to the next-to-leading order perturbative QCD prediction and various other standard model predictions.

  8. Improving activation cross section data with TALYS

    NASA Astrophysics Data System (ADS)

    Dzysiuk, Nataliia; Koning, Arjan

    2017-09-01

    Needs for accurate (n,x) activation cross sections for fusion technology have been considered with reference to the current status of the TENDL library. The current work is focused on improving activation cross section data for nuclear reactions relevant mainly for fusion and astrophysical needs. The fits have been performed with the TALYS-1.8 code by means of nuclear model parameter variation, mostly for the optical model and level densities, followed by comparison to recent experimental data taken from EXFOR and other evaluated nuclear databases. The updated cross section data are going to be adopted into the new version of TENDL. The improvements have been performed both for differential as well as integral data sets.

  9. Covariance Evaluation Methodology for Neutron Cross Sections

    SciTech Connect

    Herman,M.; Arcilla, R.; Mattoon, C.M.; Mughabghab, S.F.; Oblozinsky, P.; Pigni, M.; Pritychenko, b.; Songzoni, A.A.

    2008-09-01

    We present the NNDC-BNL methodology for estimating neutron cross section covariances in thermal, resolved resonance, unresolved resonance and fast neutron regions. The three key elements of the methodology are Atlas of Neutron Resonances, nuclear reaction code EMPIRE, and the Bayesian code implementing Kalman filter concept. The covariance data processing, visualization and distribution capabilities are integral components of the NNDC methodology. We illustrate its application on examples including relatively detailed evaluation of covariances for two individual nuclei and massive production of simple covariance estimates for 307 materials. Certain peculiarities regarding evaluation of covariances for resolved resonances and the consistency between resonance parameter uncertainties and thermal cross section uncertainties are also discussed.

  10. New Parameterization of Neutron Absorption Cross Sections

    NASA Technical Reports Server (NTRS)

    Tripathi, Ram K.; Wilson, John W.; Cucinotta, Francis A.

    1997-01-01

    Recent parameterization of absorption cross sections for any system of charged ion collisions, including proton-nucleus collisions, is extended for neutron-nucleus collisions valid from approx. 1 MeV to a few GeV, thus providing a comprehensive picture of absorption cross sections for any system of collision pairs (charged or uncharged). The parameters are associated with the physics of the problem. At lower energies, optical potential at the surface is important, and the Pauli operator plays an increasingly important role at intermediate energies. The agreement between the calculated and experimental data is better than earlier published results.

  11. Infrared absorption cross sections of alternative CFCs

    NASA Technical Reports Server (NTRS)

    Clerbaux, Cathy; Colin, Reginald; Simon, Paul C.

    1994-01-01

    Absorption cross sections have obtained in the infrared atmospheric window, between 600 and 1500 cm(exp -1), for 10 alternative hydrohalocarbons: HCFC-22, HCFC-123, HCFC-124, HCFC-141b, HCFC-142b, HCFC-225ca, HCFC-225cb, HFC-125, HFC-134a, and HFC-152a. The measurements were made at three temperatures (287K, 270K and 253K) with a Fourier transform spectrometer operating at 0.03 cm(exp -1) apodized resolution. Integrated cross sections are also derived for use in radiative models to calculate the global warming potentials.

  12. Cross section for 246Cm subbarrier fission

    NASA Astrophysics Data System (ADS)

    Alekseev, A. A.; Bergman, A. A.; Berlev, A. I.; Koptelov, E. A.; Samylin, B. F.; Trufanov, A. M.; Fursov, B. I.; Shorin, V. S.

    2010-10-01

    The cross section for 246Cm fission induced by neutrons of energy in the range 0.1 eV-20 keV was measured by the neutron lead slowing-down spectrometer (LSDS-100) of the Institute for Nuclear Research (INR, Russian Academy of Sciences, Moscow). The parameters of the resonance area and of the fission width were evaluated for several low-lying s-wave neutron resonances. The parameters of the intermediate structure in the cross section for the subbarrier fusion of 246Cm nuclei were found. The results obtained in this way were compared with available experimental data and with recommended evaluated data.

  13. Optical Model and Cross Section Uncertainties

    SciTech Connect

    Herman,M.W.; Pigni, M.T.; Dietrich, F.S.; Oblozinsky, P.

    2009-10-05

    Distinct minima and maxima in the neutron total cross section uncertainties were observed in model calculations using spherical optical potential. We found this oscillating structure to be a general feature of quantum mechanical wave scattering. Specifically, we analyzed neutron interaction with 56Fe from 1 keV up to 65 MeV, and investigated physical origin of the minima.We discuss their potential importance for practical applications as well as the implications for the uncertainties in total and absorption cross sections.

  14. Multigroup cross section library for GFR2400

    NASA Astrophysics Data System (ADS)

    Čerba, Štefan; Vrban, Branislav; Lüley, Jakub; Haščík, Ján; Nečas, Vladimír

    2017-09-01

    In this paper the development and optimization of the SBJ_E71 multigroup cross section library for GFR2400 applications is discussed. A cross section processing scheme, merging Monte Carlo and deterministic codes, was developed. Several fine and coarse group structures and two weighting flux options were analysed through 18 benchmark experiments selected from the handbook of ICSBEP and based on performed similarity assessments. The performance of the collapsed version of the SBJ_E71 library was compared with MCNP5 CE ENDF/B VII.1 and the Korean KAFAX-E70 library. The comparison was made based on integral parameters of calculations performed on full core homogenous models.

  15. New Parameterization of Neutron Absorption Cross Sections

    NASA Astrophysics Data System (ADS)

    Tripathi, Ram K.; Wilson, John W.; Cucinotta, Francis A.

    1997-06-01

    Recent parameterization of absorption cross sections for any system of charged ion collisions, including proton-nucleus collisions, is extended for neutron-nucleus collisions valid from approx. 1 MeV to a few GeV, thus providing a comprehensive picture of absorption cross sections for any system of collision pairs (charged or uncharged). The parameters are associated with the physics of the problem. At lower energies, optical potential at the surface is important, and the Pauli operator plays an increasingly important role at intermediate energies. The agreement between the calculated and experimental data is better than earlier published results.

  16. Precise neutron inelastic cross section measurements

    SciTech Connect

    Negret, Alexandru

    2012-11-20

    The design of a new generation of nuclear reactors requires the development of a very precise neutron cross section database. Ongoing experiments performed at dedicated facilities aim to the measurement of such cross sections with an unprecedented uncertainty of the order of 5% or even smaller. We give an overview of such a facility: the Gamma Array for Inelastic Neutron Scattering (GAINS) installed at the GELINA neutron source of IRMM, Belgium. Some of the most challenging difficulties of the experimental approach are emphasized and recent results are shown.

  17. Universal Parameterization of Absorption Cross Sections

    NASA Technical Reports Server (NTRS)

    Tripathi, R. K.; Cucinotta, Francis A.; Wilson, John W.

    1999-01-01

    Our prior nuclear absorption cross sections model is extended for light systems (A less than or equal to 4) where either both projectile and target are light particles or one is a light particle and the other is a medium or heavy nucleus. The agreement with experiment is excellent for these cases as well. Present work in combination with our original model provides a comprehensive picture of absorption cross sections for light, medium, and heavy systems, a very valuable input for radiation protection studies.

  18. Neutron Capture Cross Section of 239Pu

    NASA Astrophysics Data System (ADS)

    Mosby, S.; Arnold, C.; Bredeweg, T. A.; Couture, A.; Jandel, M.; O'Donnell, J. M.; Rusev, G.; Ullmann, J. L.; Chyzh, A.; Henderson, R.; Kwan, E.; Wu, C. Y.

    2014-09-01

    The 239Pu(n,γ) cross section has been measured over the energy range 10 eV - 10 keV using the Detector for Advanced Neutron Capture Experiments (DANCE) as part of a campaign to produce precision (n,γ) measurements on 239Pu in the keV region. Fission coincidences were measured with a PPAC and used to characterize the prompt fission γ-ray spectrum in this region. The resulting spectra will be used to better characterize the fission component of another experiment with a thicker target to extend the (n,γ) cross section measurement well into the keV region.

  19. Total cross sections for +/-atom collisions

    NASA Astrophysics Data System (ADS)

    Gien, T. T.

    1987-03-01

    The total cross sections for electron and positron scatterings by lithium, sodium, and potassium in the intermediate energy range from 40 to 1000 eV are calculated using the modified Glauber and second Born approximations. A model potential approach is developed to enable an exact inclusion of the core-interaction effects. Within this approach, the positron cross sections are predicted to be somewhat smaller than those of electron scattering. Calculations have also been performed with the consideration of the inert-core and frozen-core assumption and the use of the Clementi wave function to represent the target electrons. Comparison to existing experimental data is made.

  20. Microscopic description of production cross sections including deexcitation effects

    NASA Astrophysics Data System (ADS)

    Sekizawa, Kazuyuki

    2017-07-01

    Background: At the forefront of the nuclear science, production of new neutron-rich isotopes is continuously pursued at accelerator laboratories all over the world. To explore the currently unknown territories in the nuclear chart far away from the stability, reliable theoretical predictions are inevitable. Purpose: To provide a reliable prediction of production cross sections taking into account secondary deexcitation processes, both particle evaporation and fission, a new method called TDHF+GEMINI is proposed, which combines the microscopic time-dependent Hartree-Fock (TDHF) theory with a sophisticated statistical compound-nucleus deexcitation model, GEMINI++. Methods: Low-energy heavy ion reactions are described based on three-dimensional Skyrme-TDHF calculations. Using the particle-number projection method, production probabilities, total angular momenta, and excitation energies of primary reaction products are extracted from the TDHF wave function after collision. Production cross sections for secondary reaction products are evaluated employing GEMINI++. Results are compared with available experimental data and widely used grazing calculations. Results: The method is applied to describe cross sections for multinucleon transfer processes in 40Ca+124Sn (Ec .m .≃128.54 MeV ), 48Ca+124Sn (Ec .m .≃125.44 MeV ), 40Ca+208Pb (Ec .m .≃208.84 MeV ), 58Ni+208Pb (Ec .m .≃256.79 MeV ), 64Ni+238U (Ec .m .≃307.35 MeV ), and 136Xe+198Pt (Ec .m .≃644.98 MeV ) reactions at energies close to the Coulomb barrier. It is shown that the inclusion of secondary deexcitation processes, which are dominated by neutron evaporation in the present systems, substantially improves agreement with the experimental data. The magnitude of the evaporation effects is very similar to the one observed in grazing calculations. TDHF+GEMINI provides better description of the absolute value of the cross sections for channels involving transfer of more than one proton, compared to the grazing

  1. Comprehensive Amm242 neutron-induced reaction cross sections and resonance parameters

    NASA Astrophysics Data System (ADS)

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; Bucher, B.; Wimer, N.; Chyzh, A.; Bredeweg, T. A.; Baramsai, B.; Couture, A.; Jandel, M.; Mosby, S.; Ullmann, J. L.

    2017-06-01

    The 242Am metastable isomer's neutron-induced destruction mechanisms were studied at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array with a compact parallel-plate avalanche counter. New Amm242 neutron-capture cross sections were determined from 100 meV to 10 keV, and the absolute scale was set with respect to a concurrent measurement of the well-known Amm242 neutron-induced-fission cross section. The new fission cross section spans an energy range from 100 meV to 1 MeV and was normalized to the ENDF/B-VII.1 evaluated cross section to set the absolute scale. Our Amm242(n ,f ) cross section agrees well with the cross section of Browne et al. [Phys. Rev. C 29, 2188 (1984)], 10.1103/PhysRevC.29.2188 over this large energy interval. The new neutron-capture cross section measurement complements and agrees well with our recent results reported below 1 eV in Buckner et al. [Phys. Rev. C 95, 024610 (2017)], 10.1103/PhysRevC.95.024610. This new work comprises the most comprehensive study of Amm242(n ,γ ) above thermal energy. Neutron-induced resonance energies and parameters were deduced with the sammy R -matrix code for incident neutron energies up to 45 eV, and the new average Γγ is 13 % higher than the evaluated average γ width.

  2. Photoionization of ClII

    NASA Astrophysics Data System (ADS)

    Nahar, Sultana; Hernández, E.; Antillón, A.; Morales, A.; González, O.; Macaluso, D.; Hanstorp, D.; Aguilar, A.; Juárez, A.; Hinojosa, G.

    2014-05-01

    The cross section and spectrum for the process of single photoionization of the chlorine cation was measured in the energy range of 19.5 to 28.0 eV with a photon energy resolution of 20 meV. Over a non resonant cross section, resonant structures originated from initinal Cl+ 3P(J=0,1,2) manifold converging mainly to 2P(J=3/2) and 2D(J=5/2) are identified. A theoretical calculation based on the close coupling R-matrix is under progress. CONACYT CB-2011 167631. US National Science Fundation, DGAPA IN106813, The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. DOE Cntrct. DE-AC02-05CH11231. Montana Space Grant Consortium, Swedish Research Council.

  3. 46 CFR 64.25 - Cross section.

    Code of Federal Regulations, 2013 CFR

    2013-10-01

    ... 46 Shipping 2 2013-10-01 2013-10-01 false Cross section. 64.25 Section 64.25 Shipping COAST GUARD, DEPARTMENT OF HOMELAND SECURITY (CONTINUED) MARINE ENGINEERING MARINE PORTABLE TANKS AND CARGO HANDLING...) Circular; or (b) Other than circular and stress analyzed experimentally by the method contained in UG-101...

  4. 46 CFR 64.25 - Cross section.

    Code of Federal Regulations, 2012 CFR

    2012-10-01

    ... 46 Shipping 2 2012-10-01 2012-10-01 false Cross section. 64.25 Section 64.25 Shipping COAST GUARD, DEPARTMENT OF HOMELAND SECURITY (CONTINUED) MARINE ENGINEERING MARINE PORTABLE TANKS AND CARGO HANDLING...) Circular; or (b) Other than circular and stress analyzed experimentally by the method contained in UG-101...

  5. Cross Sections From Scalar Field Theory

    NASA Technical Reports Server (NTRS)

    Norbury, John W.; Dick, Frank; Norman, Ryan B.; Nasto, Rachel

    2008-01-01

    A one pion exchange scalar model is used to calculate differential and total cross sections for pion production through nucleon- nucleon collisions. The collisions involve intermediate delta particle production and decay to nucleons and a pion. The model provides the basic theoretical framework for scalar field theory and can be applied to particle production processes where the effects of spin can be neglected.

  6. Reaction cross section of 22C

    NASA Astrophysics Data System (ADS)

    Togano, Yasuhiro; Samurai Collaboration

    2014-09-01

    Reaction cross section of 22C on a carbon target at an energy of 240 MeV/nucleon have been measured by using the transmission method. The most neutron-rich carbon isotopes 22C is a candidate of a two-neutron halo nucleus. Tanaka et al. [1] measured the reaction cross section of 22C on a hydrogen target at 40 MeV/nucleon. It is showed 22C to have a large matter radius of 5 . 9 +/- 0 . 9 fm, which is much larger than the ones of carbon isotopes with N <= 14 , suggesting 22C is the halo nucleus. This reported radius has a large uncertainty due to a lack of statistics. To deduce a more accurate matter radius of 22C, the measurement of reaction cross section with higher statistics at a higher beam energy are required. The experiment was performed by using the SAMURAI spectrometer at RIBF. The 22C beam at 240 MeV/nucleon was impinged on a carbon target, and the reaction product was identified by using SAMURAI spectrometer. In the present talk, the extracted reaction cross section and derived matter density distribution of 22C will be presented.

  7. Cotton fibre cross-section properties

    USDA-ARS?s Scientific Manuscript database

    From a structural perspective the cotton fibre is a singularly discrete, elongated plant cell with no junctions or inter-cellular boundaries. Its form in nature is essentially unadulterated from the field to the spinning mill where its cross-section properties, as for any textile fibre, are central ...

  8. Photoelectric absorption cross sections with variable abundances

    NASA Technical Reports Server (NTRS)

    Balucinska-Church, Monika; Mccammon, Dan

    1992-01-01

    Polynomial fit coefficients have been obtained for the energy dependences of the photoelectric absorption cross sections of 17 astrophysically important elements. These results allow the calculation of X-ray absorption in the energy range 0.03-10 keV in material with noncosmic abundances.

  9. Cross-sectional structural parameters from densitometry

    NASA Technical Reports Server (NTRS)

    Cleek, Tammy M.; Whalen, Robert T.

    2002-01-01

    Bone densitometry has previously been used to obtain cross-sectional properties of bone from a single X-ray projection across the bone width. Using three unique projections, we have extended the method to obtain the principal area moments of inertia and orientations of the principal axes at each scan cross-section along the length of the scan. Various aluminum phantoms were used to examine scanner characteristics to develop the highest accuracy possible for in vitro non-invasive analysis of cross-sectional properties. Factors considered included X-ray photon energy, initial scan orientation, the angle spanned by the three scans (included angle), and I(min)/I(max) ratios. Principal moments of inertia were accurate to within +/-3.1% and principal angles were within +/-1 degrees of the expected value for phantoms scanned with included angles of 60 degrees and 90 degrees at the higher X-ray photon energy (140 kVp). Low standard deviations in the error (0.68-1.84%) also indicate high precision of calculated measurements with these included angles. Accuracy and precision decreased slightly when the included angle was reduced to 30 degrees. The method was then successfully applied to a pair of excised cadaveric tibiae. The accuracy and insensitivity of the algorithms to cross-sectional shape and changing isotropy (I(min)/I(max)) values when various included angles are used make this technique viable for future in vivo studies.

  10. Cross-sectional structural parameters from densitometry

    NASA Technical Reports Server (NTRS)

    Cleek, Tammy M.; Whalen, Robert T.

    2002-01-01

    Bone densitometry has previously been used to obtain cross-sectional properties of bone from a single X-ray projection across the bone width. Using three unique projections, we have extended the method to obtain the principal area moments of inertia and orientations of the principal axes at each scan cross-section along the length of the scan. Various aluminum phantoms were used to examine scanner characteristics to develop the highest accuracy possible for in vitro non-invasive analysis of cross-sectional properties. Factors considered included X-ray photon energy, initial scan orientation, the angle spanned by the three scans (included angle), and I(min)/I(max) ratios. Principal moments of inertia were accurate to within +/-3.1% and principal angles were within +/-1 degrees of the expected value for phantoms scanned with included angles of 60 degrees and 90 degrees at the higher X-ray photon energy (140 kVp). Low standard deviations in the error (0.68-1.84%) also indicate high precision of calculated measurements with these included angles. Accuracy and precision decreased slightly when the included angle was reduced to 30 degrees. The method was then successfully applied to a pair of excised cadaveric tibiae. The accuracy and insensitivity of the algorithms to cross-sectional shape and changing isotropy (I(min)/I(max)) values when various included angles are used make this technique viable for future in vivo studies.

  11. Neutron capture cross section of Am241

    NASA Astrophysics Data System (ADS)

    Jandel, M.; Bredeweg, T. A.; Bond, E. M.; Chadwick, M. B.; Clement, R. R.; Couture, A.; O'Donnell, J. M.; Haight, R. C.; Kawano, T.; Reifarth, R.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Wouters, J. M.; Agvaanluvsan, U.; Parker, W. E.; Wu, C. Y.; Becker, J. A.

    2008-09-01

    The neutron capture cross section of Am241 for incident neutrons from 0.02 eV to 320 keV has been measured with the detector for advanced neutron capture experiments (DANCE) at the Los Alamos Neutron Science Center. The thermal neutron capture cross section was determined to be 665±33 b. Our result is in good agreement with other recent measurements. Resonance parameters for En<12 eV were obtained using an R-matrix fit to the measured cross section. The results are compared with values from the ENDF/B-VII.0, Mughabghab, JENDL-3.3, and JEFF-3.1 evaluations. Γn neutron widths for the first three resonances are systematically larger by 5-15% than the ENDF/B-VII.0 values. The resonance integral above 0.5 eV was determined to be 1553±7 b. Cross sections in the resolved and unresolved energy regions above 12 eV were calculated using the Hauser-Feshbach theory incorporating the width-fluctuation correction of Moldauer. The calculated results agree well with the measured data, and the extracted averaged resonance parameters in the unresolved resonance region are consistent with those for the resolved resonances.

  12. Testing (Validating?) Cross Sections with ICSBEP Benchmarks

    SciTech Connect

    Kahler, Albert C. III

    2012-06-28

    We discuss how to use critical benchmarks from the International Handbook of Evaluated Criticality Safety Benchmark Experiments to determine the applicability of specific cross sections to the end-user's problem of interest. Particular attention is paid to making sure the selected suite of benchmarks includes the user's range of applicability (ROA).

  13. Future experimental programme for neutrino cross sections

    NASA Astrophysics Data System (ADS)

    Bolognesi, Sara

    2017-09-01

    The neutrino-nucleus interaction modelling is crucial for a precise measurement of neutrino oscillations. The advantages and the drawbacks of the planned strategies to measure the neutrino-nucleus cross section with different detector technologies will be discussed. The present document summarizes a talk given on these topics at Neutrino 2016 conference.

  14. Measurement of the Am242m neutron-induced reaction cross sections

    DOE PAGES

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; ...

    2017-02-17

    The neutron-induced reaction cross sections of 242mAm were measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. A new neutron-capture cross section was determined, and the absolute scale was set according to a concurrent measurement of the well-known 242mAm(n,f) cross section. The (n,γ) cross section was measured from thermal energy to an incident energy of 1 eV at which point the data quality was limited by the reaction yield in the laboratory. Our new 242mAm fission cross section was normalized to ENDF/B-VII.1 tomore » set the absolute scale, and it agreed well with the (n,f) cross section from thermal energy to 1 keV. Lastly, the average absolute capture-to-fission ratio was determined from thermal energy to En = 0.1 eV, and it was found to be 26(4)% as opposed to the ratio of 19% from the ENDF/B-VII.1 evaluation.« less

  15. Measurement of the Amm242 neutron-induced reaction cross sections

    NASA Astrophysics Data System (ADS)

    Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; Bucher, B.; Wimer, N.; Chyzh, A.; Bredeweg, T. A.; Baramsai, B.; Couture, A.; Jandel, M.; Mosby, S.; Ullmann, J. L.; Dance Collaboration

    2017-02-01

    The neutron-induced reaction cross sections of Amm242 were measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. A new neutron-capture cross section was determined, and the absolute scale was set according to a concurrent measurement of the well-known Amm242(n ,f ) cross section. The (n ,γ ) cross section was measured from thermal energy to an incident energy of 1 eV at which point the data quality was limited by the reaction yield in the laboratory. Our new Amm242 fission cross section was normalized to ENDF/B-VII.1 to set the absolute scale, and it agreed well with the (n ,f ) cross section reported by Browne et al. (1984) from thermal energy to 1 keV. The average absolute capture-to-fission ratio was determined from thermal energy to En=0.1 eV, and it was found to be 26(4)% as opposed to the ratio of 19 % from the ENDF/B-VII.1 evaluation.

  16. The Elusive p-air cross section

    NASA Astrophysics Data System (ADS)

    Block, M. M.

    2006-09-01

    For the $\\pbar p$ and $pp$ systems, we have used all of the extensive data of the Particle Data Group[K. Hagiwara {\\em et al.} (Particle Data Group), Phys. Rev. D 66, 010001 (2002).]. We then subject these data to a screening process, the ``Sieve'' algorithm[M. M. Block, physics/0506010.], in order to eliminate ``outliers'' that can skew a $\\chi^2$ fit. With the ``Sieve'' algorithm, a robust fit using a Lorentzian distribution is first made to all of the data to sieve out abnormally high $\\delchi$, the individual i$^{\\rm th}$ point's contribution to the total $\\chi^2$. The $\\chi^2$ fits are then made to the sieved data. We demonstrate that we cleanly discriminate between asymptotic $\\ln s$ and $\\ln^2s$ behavior of total hadronic cross sections when we require that these amplitudes {\\em also} describe, on average, low energy data dominated by resonances. We simultaneously fit real analytic amplitudes to the ``sieved'' high energy measurements of $\\bar p p$ and $pp$ total cross sections and $\\rho$-values for $\\sqrt s\\ge 6$ GeV, while requiring that their asymptotic fits smoothly join the the $\\sigma_{\\bar p p}$ and $\\sigma_{pp}$ total cross sections at $\\sqrt s=$4.0 GeV--again {\\em both} in magnitude and slope. Our results strongly favor a high energy $\\ln^2s$ fit, basically excluding a $\\ln s$ fit. Finally, we make a screened Glauber fit for the p-air cross section, using as input our precisely-determined $pp$ cross sections at cosmic ray energies.

  17. Gadolinium photoionization process

    DOEpatents

    Paisner, Jeffrey A.; Comaskey, Brian J.; Haynam, Christopher A.; Eggert, Jon H.

    1993-01-01

    A method is provided for selective photoionization of the odd-numbered atomic mass gadolinium isotopes 155 and 157. The selective photoionization is accomplished by circular or linear parallel polarized laser beam energy effecting a three-step photoionization pathway.

  18. Gadolinium photoionization process

    DOEpatents

    Paisner, J.A.; Comaskey, B.J.; Haynam, C.A.; Eggert, J.H.

    1993-04-13

    A method is provided for selective photoionization of the odd-numbered atomic mass gadolinium isotopes 155 and 157. The selective photoionization is accomplished by circular or linear parallel polarized laser beam energy effecting a three-step photoionization pathway.

  19. Two-photon standard technique for measuring the two-photon absorption cross section in complex organic molecules

    SciTech Connect

    Alfimov, E.E.; Groshev, D.E.; Makukha, V.K.; Meshalkin, Y.P.

    1995-03-01

    The two-photon standard technique for measuring the absolute cross sections for two-photon absorption of complex organic molecules is proposed, which is quite insensitive to the spatial and temporal fluctuations of the laser beam. n-Bismethylsterilbenzene (MSB) with a known value of the two-photon absorption cross section is used as a standard. 9 refs., 2 figs.

  20. Dynamics of photoionization of hydrogenlike ions in Debye plasmas

    SciTech Connect

    Qi, Y. Y.; Wang, J. G.; Janev, R. K.

    2009-12-15

    Photoionization processes for the ground state and n<=3 excited states of hydrogenlike ions embedded in a weakly coupled plasma are investigated in the entire energy range of a nonrelativistic regime. The plasma screening of the Coulomb interaction between charged particles is described by the Debye-Hueckel model. The energy levels and wave functions for both the bound and continuum states are calculated by solving the Schroedinger equation numerically by the symplectic integrator. The screening of Coulomb interactions reduces the number of bound electron states, decreases their binding energies, broadens the radial distribution of electron wave functions of these states, and changes significantly the phases and the amplitudes of continuum wave functions. These changes strongly affect the dipole matrix elements between the bound and continuum states and, hence, the photoionization cross sections. The most significant effects of the screened Coulomb interactions on the energy behavior of photoionization cross sections are manifested in its low-energy behavior (Wigner threshold law), the appearance of multiple shape and virtual-state resonances when the energy levels of upper bound states enter the continuum after certain critical strength of the screening, and in the (slight) reduction of the cross section at high photon energies. All these features of the photoionization cross section are related to the short-range character of the Debye-Hueckel potential. The effects of the potential screening on the Combet-Farnoux and Cooper minima in the photoionization cross section are also investigated. Comparison of calculated photoionization cross sections with the results of other authors, when available, is made.

  1. Tables of nuclear cross sections for galactic cosmic rays: Absorption cross sections

    NASA Technical Reports Server (NTRS)

    Townsend, L. W.; Wilson, J. W.

    1985-01-01

    A simple but comprehensive theory of nuclear reactions is presented. Extensive tables of nucleon, deuteron, and heavy-ion absorption cross sections over a broad range of energies are generated for use in cosmic ray shielding studies. Numerous comparisons of the calculated values with available experimental data show agreement to within 3 percent for energies above 80 MeV/nucleon and within approximately 10 percent for energies as low as 30 MeV/nucleon. These tables represent the culmination of the development of the absorption cross section formalism and supersede the preliminary absorption cross sections published previously in NASA TN D-8107, NASA TP-2138, and NASA TM-84636.

  2. Tables of nuclear cross sections for galactic cosmic rays: Absorption cross sections

    NASA Astrophysics Data System (ADS)

    Townsend, L. W.; Wilson, J. W.

    1985-05-01

    A simple but comprehensive theory of nuclear reactions is presented. Extensive tables of nucleon, deuteron, and heavy-ion absorption cross sections over a broad range of energies are generated for use in cosmic ray shielding studies. Numerous comparisons of the calculated values with available experimental data show agreement to within 3 percent for energies above 80 MeV/nucleon and within approximately 10 percent for energies as low as 30 MeV/nucleon. These tables represent the culmination of the development of the absorption cross section formalism and supersede the preliminary absorption cross sections published previously in NASA TN D-8107, NASA TP-2138, and NASA TM-84636.

  3. Measurement of electron-attachment line shapes, cross sections, and rate constants in HI and DI at ultralow electron energies

    NASA Technical Reports Server (NTRS)

    Alajajian, S. H.; Chutjian, A.

    1988-01-01

    Electron-attachment cross sections are reported in the electron energy range 0-150 MeV, at an energy resolution of 6.5 MeV (full width at half maximum) for the molecules HI and DI. Use is made of the Kr photoionization method to obtain cross sections for HI, and a signal intercomparison technique to obtain cross sections and the thermal-attachment rate constant for DI. Attachment properties of the two molecules are very similar. The ratio of attachment cross sections is discussed in terms of the reduced-mass dependence of the dissociation width and the survival probability, and in terms of spectroscopic thresholds and rotational populations for attachment at 300 K. Approximate potential-energy curves for the lowest states of the neutral molecule and negative ion are given.

  4. Rotational averaging of multiphoton absorption cross sections

    NASA Astrophysics Data System (ADS)

    Friese, Daniel H.; Beerepoot, Maarten T. P.; Ruud, Kenneth

    2014-11-01

    Rotational averaging of tensors is a crucial step in the calculation of molecular properties in isotropic media. We present a scheme for the rotational averaging of multiphoton absorption cross sections. We extend existing literature on rotational averaging to even-rank tensors of arbitrary order and derive equations that require only the number of photons as input. In particular, we derive the first explicit expressions for the rotational average of five-, six-, and seven-photon absorption cross sections. This work is one of the required steps in making the calculation of these higher-order absorption properties possible. The results can be applied to any even-rank tensor provided linearly polarized light is used.

  5. Rotational averaging of multiphoton absorption cross sections.

    PubMed

    Friese, Daniel H; Beerepoot, Maarten T P; Ruud, Kenneth

    2014-11-28

    Rotational averaging of tensors is a crucial step in the calculation of molecular properties in isotropic media. We present a scheme for the rotational averaging of multiphoton absorption cross sections. We extend existing literature on rotational averaging to even-rank tensors of arbitrary order and derive equations that require only the number of photons as input. In particular, we derive the first explicit expressions for the rotational average of five-, six-, and seven-photon absorption cross sections. This work is one of the required steps in making the calculation of these higher-order absorption properties possible. The results can be applied to any even-rank tensor provided linearly polarized light is used.

  6. Universal Parameterization of Absorption Cross Sections

    NASA Technical Reports Server (NTRS)

    Tripathi, R. K.; Cucinotta, Francis A.; Wilson, John W.

    1997-01-01

    This paper presents a simple universal parameterization of total reaction cross sections for any system of colliding nuclei that is valid for the entire energy range from a few AMeV to a few AGeV. The universal picture presented here treats proton-nucleus collision as a special case of nucleus-nucleus collision, where the projectile has charge and mass number of one. The parameters are associated with the physics of the collision system. In general terms, Coulomb interaction modifies cross sections at lower energies, and the effects of Pauli blocking are important at higher energies. The agreement between the calculated and experimental data is better than all earlier published results.

  7. Proton Pair Production Cross Sections at BESIII

    NASA Astrophysics Data System (ADS)

    Zhou, Xiaorong

    Using data samples collected with the BESIII detector at the BEPCII collider, the Born cross section of e + e - to pbar{p} at 12 center-of-mass energies from 2232.4 to 3671.0 MeV is provided. The corresponding effective electromagnetic form factor of the proton is deduced under the assumption that the electric and magnetic form factors are equal. In addition, the ratio of electric to magnetic form factors are extracted for the data samples with larger statistics. The measured cross sections are in agreement with recent results from BaBar, improving the overall uncertainty by about 30%. The |GE/GM| ratios are close to unity and consistent with BaBar results in the same q2 region.

  8. Extinction cross section of a dielectric strip

    NASA Astrophysics Data System (ADS)

    Dowerah, Subratananda; Chakrabarti, Aloknath

    1988-05-01

    The problem of scattering of a plane electromagnetic wave by a dielectric strip is formulated in terms of an uncoupled system of three-part Wiener-Hopf equations by using a set of approximate boundary conditions derived and utilized recently. The resulting Wiener-Hopf problems are solved approximately for sufficiently large values of the width of the strip by using Jones' method (1964). An analytical formula is derived for the excitation cross section of the strip under consideration from which numerical values are obtained in specific situations and the results are presented graphically. The radar cross section of the strip is also computed for several special circumstances and these are presented separately.

  9. Sketching cross sections with a portable microcomputer

    SciTech Connect

    Kimberley, M.M.

    1985-02-01

    Computer applications have been carried to the field long ago by geophysicists and their dog houses. The advent of inexpensive battery-powered microcomputers promises to allow the field geologist to participate in this application. The field geologist may record data directly onto a computer-readable medium and calculate statistics or plot a cross section. A program for routine plotting of cross sections in the field has been developed and field-tested. The program proved to be useful to 30 computer-illiterate geologists on a 6-week mapping project in New Mexico. The program allows the user to control vertical exaggeration and displays the correct apparent dip along the chosen line of section. Cubic-spline interpolation is used to plot both topography and folded bedding planes. The program executes in Pascal on an Apple IIc in a few seconds.

  10. Double-photoionization of helium including quadrupole radiation effects

    SciTech Connect

    Colgan, James; Ludlow, J A; Lee, Teck - Ghee; Pindzola, M S; Robicheaux, F

    2009-01-01

    Non-perturbative time-dependent close-coupling calculations are carried out for the double photoionization of helium including both dipole and quadrupole radiation effects. At a photon energy of 800 eV, accessible at CUlTent synchrotron light sources, the quadrupole interaction contributes around 6% to the total integral double photoionization cross section. The pure quadrupole single energy differential cross section shows a local maxima at equal energy sharing, as opposed to the minimum found in the pure dipole single energy differential cross section. The sum of the pure dipole and pure quadrupole single energy differentials is insensitive to non-dipole effects at 800 eV. However, the triple differential cross section at equal energy sharing of the two ejected electrons shows strong non-dipole effects due to the quadrupole interaction that may be experimentally observable.

  11. Fusion cross sections measurements with MUSIC

    NASA Astrophysics Data System (ADS)

    Carnelli, P. F. F.; Fernández Niello, J. O.; Almaraz-Calderon, S.; Rehm, K. E.; Albers, M.; Digiovine, B.; Esbensen, H.; Henderson, D.; Jiang, C. L.; Nusair, O.; Palchan-Hazan, T.; Pardo, R. C.; Ugalde, C.; Paul, M.; Alcorta, M.; Bertone, P. F.; Lai, J.; Marley, S. T.

    2014-09-01

    The interaction between exotic nuclei plays an important role for understanding the reaction mechanism of the fusion processes as well as for the energy production in stars. With the advent of radioactive beams new frontiers for fusion reaction studies have become accessible. We have performed the first measurements of the total fusion cross sections in the systems 10 , 14 , 15C + 12C using a newly developed active target-detector system (MUSIC). Comparison of the obtained cross sections with theoretical predictions show a good agreement in the energy region accessible with existing radioactive beams. This type of comparison allows us to calibrate the calculations for cases that cannot be studied in the laboratory with the current experimental capabilities. The high efficiency of this active detector system will allow future measurements with even more neutron-rich isotopes. The interaction between exotic nuclei plays an important role for understanding the reaction mechanism of the fusion processes as well as for the energy production in stars. With the advent of radioactive beams new frontiers for fusion reaction studies have become accessible. We have performed the first measurements of the total fusion cross sections in the systems 10 , 14 , 15C + 12C using a newly developed active target-detector system (MUSIC). Comparison of the obtained cross sections with theoretical predictions show a good agreement in the energy region accessible with existing radioactive beams. This type of comparison allows us to calibrate the calculations for cases that cannot be studied in the laboratory with the current experimental capabilities. The high efficiency of this active detector system will allow future measurements with even more neutron-rich isotopes. This work is supported by the U.S. DOE Office of Nuclear Physics under Contract No. DE-AC02-06CH11357 and the Universidad Nacional de San Martin, Argentina, Grant SJ10/39.

  12. Fusion cross sections and the new dynamics

    SciTech Connect

    Swiatecki, W.J.

    1981-05-01

    The prediction of the need for an extra push over the interaction barrier in order to make the heavier nuclei fuse is made the basis of a simple algebraic theory for the energy-dependence of the fusion cross-section. A comparison with recent experiments promises to provide a quantitative test of the New Dynamics (the theory of macroscopic nuclear shape evolutions based on the one-body dissipation concept).

  13. {sup 231}Pa photofission cross section

    SciTech Connect

    Soldatov, A.S.; Rudnikov, V.E.; Smirenkin, G.N.

    1995-12-01

    The measurements of the {sup 231}Pa yield and cross section photofission in the energy range 7-9 MeV are presented. These measurements are a continuation of similar measurements performed for the {gamma}-ray energy range 4.8-7 MeV. The entire collection of experimental data which combine the results obtained in the present work and in Ref. 1 was analyzed.

  14. How to Calculate Colourful Cross Sections Efficiently

    SciTech Connect

    Gleisberg, Tanju; Hoeche, Stefan; Krauss, Frank

    2008-09-03

    Different methods for the calculation of cross sections with many QCD particles are compared. To this end, CSW vertex rules, Berends-Giele recursion and Feynman-diagram based techniques are implemented as well as various methods for the treatment of colours and phase space integration. We find that typically there is only a small window of jet multiplicities, where the CSW technique has efficiencies comparable or better than both of the other two methods.

  15. Inclusive jet cross section at D0

    SciTech Connect

    Bhattacharjee, M.

    1996-09-01

    Preliminary measurement of the central ({vert_bar}{eta}{vert_bar} {<=} 0.5) inclusive jet cross sections for jet cone sizes of 1.0, 0.7, and 0.5 at D{null} based on the 1992-1993 (13.7 {ital pb}{sup -1}) and 1994-1995 (90 {ital pb}{sup -1}) data samples are presented. Comparisons to Next-to-Leading Order (NLO) Quantum Chromodynamics (QCD) calculations are made.

  16. Inclusive jet cross section measurement at CDF

    SciTech Connect

    Pagliarone, C.

    1996-08-01

    The CDF Collaboration has measured the inclusive jet cross section using 1992-93 collider data at 1.8 TeV. The CDF measurement is in very good agreement with NLO QCD predictions for transverse energies (E{sub T}) below 200 GeV. However, it is systematically higher than NLO QCD predictions for E{sub T} above 200 GeV.

  17. Active-beam cross-sectional modeling

    NASA Astrophysics Data System (ADS)

    Cesnik, Carlos E. S.; Ortega-Morales, Miguel

    2000-06-01

    A finite-element based analysis for modeling active composite beams with embedded anisotropic actuation is presented. It is derived from three-dimensional electroelasticity, where the original problem is reduced via the variational asymptotic method. The resulting cross-sectional analysis takes into consideration passive and active anisotropic and nonhomogeneous materials, and represents general (thin-walled, thick-walled, solid) cross-sectional geometries. The formulation requires neither the costly use of 3-D finite element discretization nor the loss of accuracy inherent to any simplified representation of the cross section. The developed formulation is numerically implemented in VABS-A, and several numerical and experimental tests cases are used to support validation of the proposed theory. Also, the effect of the presence of a core in originally hallow configurations is presented and counter-intuitive conclusions are discussed. The generality of the method and accuracy of the results increase confidence at the design stage that the active beam structure will perform as expected and, consequently, should lower costs from experimental tests and further adjustments.

  18. Quality Quantification of Evaluated Cross Section Covariances

    SciTech Connect

    Varet, S.; Dossantos-Uzarralde, P.

    2015-01-15

    Presently, several methods are used to estimate the covariance matrix of evaluated nuclear cross sections. Because the resulting covariance matrices can be different according to the method used and according to the assumptions of the method, we propose a general and objective approach to quantify the quality of the covariance estimation for evaluated cross sections. The first step consists in defining an objective criterion. The second step is computation of the criterion. In this paper the Kullback-Leibler distance is proposed for the quality quantification of a covariance matrix estimation and its inverse. It is based on the distance to the true covariance matrix. A method based on the bootstrap is presented for the estimation of this criterion, which can be applied with most methods for covariance matrix estimation and without the knowledge of the true covariance matrix. The full approach is illustrated on the {sup 85}Rb nucleus evaluations and the results are then used for a discussion on scoring and Monte Carlo approaches for covariance matrix estimation of the cross section evaluations.

  19. Nonperturbative theory of double photoionization of the hydrogen molecule

    SciTech Connect

    Vanroose, W.; Martin, F.; Rescigno, T.N.; McCurdy, C.W.

    2004-10-01

    We present completely ab initio nonperturbative calculations of the integral and single differential cross sections for double photoionization of H2 for photon energies from 53.9 to 75.7 eV. The method of exterior complex scaling, implemented with B-splines, is used to solve the Schrodinger equation for a correlated continuum wave function corresponding to a single photon having been absorbed by a correlated initial state. The results are in good agreement with experimental integral cross sections.

  20. Determination of band oscillator strengths of atmospheric molecules from high resolution vacuum ultraviolet cross section measurements

    NASA Technical Reports Server (NTRS)

    Parkinson, W. H.

    1986-01-01

    An account is given of progress in work on (1) the determination of band oscillator strengths of the Schumann-Runge absorption bands of (16)O2 and (18)O2 from cross section measurements conducted at 79 K; (2) the determination of the absolute absorption cross section of the Schumann-Runge bands of (16)O(18)O from optical depth measurements performed on mixtures of (16)O2, (18)O2 and (16)O(18)O at 79K; and (3) the influence of Schumann-Runge linewing contributions on the determination of the Herzberg continuum absorption cross section of (16)O2 in the wavelength region 194 to 204 nm. The experimental investigations are effected at high resolution with a 6.65 m scanning spectrometer which is, by virtue of its small instrumental width (EWHM = 0.0013 nm), uniquely suitable for cross section measurements of molecular bands with discrete rotational structure. Absolute cross sections, which are independent of the instrumental function and from which band oscillator strengths are directly determined, are measured for the absorption bands that are most predissociated. Such measurements are needed for (1) accurate calculations of the stratospheric production of atomic oxygen and heavy ozone formed following the photopredissociation of (18)O(16)O by solar radiation penetrating between the absorption lines of (16)O2; (2) elucidation of the mechanism of predissociation of the upper state of the Schumann-Runge bands; and (3) determination of the true shape of the Herzberg continuum cross section.

  1. K-shell ionization cross section for Ti, Fe, Cu, Zr, and Ag

    SciTech Connect

    Benka, O.; Geretschlager, M.

    1981-04-01

    Absolute K-shell ionisation cross sections have been measured for thin targets of Ti, Fe, Cu, Zr and Ag for protons in the energy range 85-790 keV and for thin targets of Ti, Fe and Cu for He ions in the energy range 190-750 keV. In addition the relative variation of the cross sections with energy has been determined with high accuracy. The experimental values are compared to the perturbed stationary state approximation (CPSSR) and the semiclassical approximation (SCA). The CPSSR theory provides the best overall agreement with experimental cross sections. For higher scaled energies the CPSSR theory predicts the energy dependence of the cross sections very well but in the lower energy range it overpredicts the cross sections by as much as a factor of two and this overprediction seems to increase with Z/sub 2/ at a fixed scaled energy y. The SCA theory predicts slightly too large ionisation cross sections except for the lowest pounds values. The relative variation of the cross sections with energy is not well described in either energy range.

  2. Capture cross section measurement analysis in the Californium-252 spectrum with the Monte Carlo method.

    PubMed

    Manojlovič, Stanko; Trkov, Andrej; Žerovnik, Gašper; Snoj, Luka

    2015-07-01

    Absolute average capture cross sections of gold, thorium, tantalum, molybdenum, copper and strontium in (252)Cf spontaneous fission neutron spectrum were simulated for two types of experiment setups preformed by Z. Dezso and J. Csikai and by L. Green. The experiments were simulated with MCNP5 using cross section data from the ENDF/B-VII.0 library. The determination of neutron backscattering was calculated with the use of neutron flagging. Correction factors to experimentally measured values were determined to obtain average cross sections in a pure (252)Cf spontaneous fission spectrum. Influence of concrete wall thickness, air moisture and room size on the average cross section was analyzed. Correction factors amounted to about 30%. Corrected values corresponding to average cross sections in a pure (252)Cf spectrum were calculated for (197)Au, (232)Th, (181)Ta, (98)Mo, (65)Cu and (84)Sr. Average cross sections were also calculated with the RR_UNC software using IRDFF-v.1.05 and ENDF/B-VII.0 libraries. The revised average radiative capture cross sections are 75.5±0.1 mb for (197)Au, 87.0±1.6 mb for (232)Th , 98.0±4.5 mb for (181)Ta, 21.2±0.5 mb for (98)Mo, 10.3±0.3 mb for (63)Cu, and 34.9±6.5 mb for (84)Sr.

  3. Measurement of electron impact collisional excitation cross sections of Ni to Ge-like gold

    NASA Astrophysics Data System (ADS)

    May, M. J.; Beiersdorfer, P.; Jordan, N.; Scofield, J. H.; Reed, K. J.; Brown, G. V.; Hansen, S. B.; Porter, F. S.; Kelley, R.; Kilbourne, C. A.; Boyce, K. R.

    2017-03-01

    We have measured the collisional excitation cross sections for the 3d→4f and 3d→5f excitations in Au ions near the Ni-like charge state by using beam plasmas created in the Livermore electron beam ion trap EBIT-I. The cross sections have been experimentally determined at approximately 1, 2 and 3 keV above the threshold energy, ET, for the 3d→4f excitations (ET ˜ 2.5 keV) and at approximately 0.1, 1 and 2 keV above the threshold energy for the 3d→5f excitations (ET ˜ 3.3 keV). The cross section measurements were made possible by using the GSFC x-ray microcalorimeter at the Livermore EBIT facility. The absolute cross sections are determined from the ratio of the intensity of the collisionally excited bound-bound transitions to the intensity of the radiative recombination lines produced in EBIT-I plasmas. The effects of polarization and Auger decay channels are accounted for in the cross section determination. Measured cross sections are compared with those from HULLAC, DWS and FAC calculations. The measurements demonstrate that some errors exist in the calculated excitation cross sections.

  4. Quantitative Collision Cross-Sections from FTICR Linewidth Measurements: Improvements in Theory and Experiment

    NASA Astrophysics Data System (ADS)

    Anupriya; Gustafson, Elaura; Mortensen, Daniel N.; Dearden, David V.

    2017-07-01

    Two corrections to the equation used in the cross-sectional areas by Fourier transform ion cyclotron resonance ("CRAFTI") technique are identified. In CRAFTI, ion collision cross-sections are obtained from the pressure-dependent ion linewidths in Fourier transform mass spectra. The effects of these corrections on the accuracy of the cross-sections obtained using the CRAFTI technique are evaluated experimentally using the 20 biogenic amino acids and several crown ether complexes with protonated alkyl monoamines. Good absolute agreement is obtained between the CRAFTI cross-sections and the corresponding cross-sections obtained using both static drift ion mobility spectrometry and computational simulations. These results indicate that the CRAFTI cross-sections obtained using the updated equation presented here are quantitatively descriptive of the size and shape of the gas-phase ions. Cross-sections that differ by less than 3% are measured for the isobaric isomers n-butylamine and tert-butylamine complexed with the crown ethers. This level of precision is similar to what has been achieved previously using traveling wave ion mobility devices. These results indicate that CRAFTI can be used to probe subtle structural differences between ions with approximately the same precision as that achieved in traveling wave ion mobility devices.

  5. Electron Bremsstrahlung Cross Sections at 25 and 50 keV from Xe and Kr

    NASA Astrophysics Data System (ADS)

    Portillo, Salvador; Quarles, C. A.

    2002-05-01

    Absolute doubly differential bremsstrahlung cross sections for radiation at 90 from 25 and 50 keV electron bombardment of Kr and Xe of will be presented. The electrons were accelerated by a Cockcroft - Walton accelerator into an Al chamber through a .06" Al collimator. Thick target bremsstrahlung background was minimized by having Al nipples and fixtures and by the addition of a carbon lined nipple placed at 180 to the SiLi detector. A comparison of the doubly differential cross sections will be made with current bremsstrahlung theories. The ratio of the Kr and Xe cross sections will also be compared with the theoretical cross section ratios. The ratio provides a more sensitive test of the contribution, if any, of polarization bremsstrahlung.

  6. Electron-impact dissociation cross sections for CHF3 and C3F8

    NASA Astrophysics Data System (ADS)

    Baio, J. E.; Yu, H.; Flaherty, D. W.; Winters, H. F.; Graves, D. B.

    2007-11-01

    Absolute total dissociation cross sections, σt,diss, by electron-impact are reported for CHF3 and C3F8 from 10 to 300 eV using the chemical gettering technique described by Winters and Inokuti (1982 Phys. Rev. A 25 1420). Data are concentrated in the near-threshold region (10-30 eV). The thresholds for dissociation of CHF3 and C3F8 are determined to be 10.4 eV and 11.9 eV, respectively. Ionization thresholds occur at 16 eV for CHF3 and 16.2 eV for C3F8. Neutral dissociation cross sections of both CHF3 and C3F8 are obtained by subtracting the ionization cross sections, σt,ion, from the total dissociation cross sections, σt,diss.

  7. Averaging cross section data so we can fit it

    SciTech Connect

    Brown, D.

    2014-10-23

    The 56Fe cross section we are interested in have a lot of fluctuations. We would like to fit the average of the cross section with cross sections calculated within EMPIRE. EMPIRE is a Hauser-Feshbach theory based nuclear reaction code, requires cross sections to be smoothed using a Lorentzian profile. The plan is to fit EMPIRE to these cross sections in the fast region (say above 500 keV).

  8. On two-parameter models of photon cross sections: application to dual-energy CT imaging.

    PubMed

    Williamson, Jeffrey F; Li, Sicong; Devic, Slobodan; Whiting, Bruce R; Lerma, Fritz A

    2006-11-01

    The goal of this study is to evaluate the theoretically achievable accuracy in estimating photon cross sections at low energies (20-1000 keV) from idealized dual-energy x-ray computed tomography (CT) images. Cross-section estimation from dual-energy measurements requires a model that can accurately represent photon cross sections of any biological material as a function of energy by specifying only two characteristic parameters of the underlying material, e.g., effective atomic number and density. This paper evaluates the accuracy of two commonly used two-parameter cross-section models for postprocessing idealized measurements derived from dual-energy CT images. The parametric fit model (PFM) accounts for electron-binding effects and photoelectric absorption by power functions in atomic number and energy and scattering by the Klein-Nishina cross section. The basis-vector model (BVM) assumes that attenuation coefficients of any biological substance can be approximated by a linear combination of mass attenuation coefficients of two dissimilar basis substances. Both PFM and BVM were fit to a modern cross-section library for a range of elements and mixtures representative of naturally occurring biological materials (Z = 2-20). The PFM model, in conjunction with the effective atomic number approximation, yields estimated the total linear cross-section estimates with mean absolute and maximum error ranges of 0.6%-2.2% and 1%-6%, respectively. The corresponding error ranges for BVM estimates were 0.02%-0.15% and 0.1%-0.5%. However, for photoelectric absorption frequency, the PFM absolute mean and maximum errors were 10.8%-22.4% and 29%-50%, compared with corresponding BVM errors of 0.4%-11.3% and 0.5%-17.0%, respectively. Both models were found to exhibit similar sensitivities to image-intensity measurement uncertainties. Of the two models, BVM is the most promising approach for realizing dual-energy CT cross-section measurement.

  9. Characterization of the Medley setup for measurements of neutron-induced fission cross sections at the GANIL-NFS facility

    NASA Astrophysics Data System (ADS)

    Tarrío, Diego; Prokofiev, Alexander V.; Gustavsson, Cecilia; Jansson, Kaj; Andersson-Sundén, Erik; Al-Adili, Ali; Pomp, Stephan

    2017-09-01

    Neutron-induced fission cross sections of 235U and 238U are widely used as standards for monitoring of neutron beams and fields. An absolute measurement of these cross sections at an absolute scale, i.e., versus the H(n,p) scattering cross section, is planned with the white neutron beam under construction at the Neutrons For Science (NFS) facility in GANIL. The experimental setup, based on PPACs and ΔE-ΔE-E telescopes containing Silicon and CsI(Tl) detectors, is described. The expected uncertainties are discussed.

  10. CCKT Calculation of e-H Total Cross Sections

    NASA Technical Reports Server (NTRS)

    Bhatia, Aaron K.; Schneider, B. I.; Temkin, A.; Fisher, Richard R. (Technical Monitor)

    2002-01-01

    We are in the process of carrying out calculations of e-H total cross sections using the 'complex-correlation Kohn-T' (CCKT) method. In a later paper, we described the methodology more completely, but confined calculations to the elastic scattering region, with definitive, precision results for S-wave phase shifts. Here we extend the calculations to the (low) continuum (1 much less than k(exp 2) much less than 3) using a Green's function formulation. This avoids having to solve integro-differential equations; rather we evaluate indefinite integrals involving appropriate Green's functions and the (complex) optical potential to find the scattering function u(r). From the asymptotic form of u(r) we extract a T(sub L) which is a complex number. From T(sub L), elastic sigma(sub L)(elastic) = 4pi(2L+1)((absolute value of T(sub L))(exp 2)), and total sigma (sub L)(total) = 4pi/k(2L+1)Im(T(sub L)) cross sections follow.

  11. CCKT Calculation of e-H Total Cross Sections

    NASA Technical Reports Server (NTRS)

    Bhatia, Aaron K.; Schneider, B. I.; Temkin, A.; Fisher, Richard R. (Technical Monitor)

    2002-01-01

    We are in the process of carrying out calculations of e-H total cross sections using the 'complex-correlation Kohn-T' (CCKT) method. In a later paper, we described the methodology more completely, but confined calculations to the elastic scattering region, with definitive, precision results for S-wave phase shifts. Here we extend the calculations to the (low) continuum (1 much less than k(exp 2) much less than 3) using a Green's function formulation. This avoids having to solve integro-differential equations; rather we evaluate indefinite integrals involving appropriate Green's functions and the (complex) optical potential to find the scattering function u(r). From the asymptotic form of u(r) we extract a T(sub L) which is a complex number. From T(sub L), elastic sigma(sub L)(elastic) = 4pi(2L+1)((absolute value of T(sub L))(exp 2)), and total sigma (sub L)(total) = 4pi/k(2L+1)Im(T(sub L)) cross sections follow.

  12. Top Production Cross Sections at D0

    SciTech Connect

    Kvita, Jiri

    2009-07-01

    We report on measurements of the ttbar production cross section at a center-of-mass energy of 1.96 TeV at the D0 experiment during Run II of the Fermilab Tevatron collider. We use candidate events in lepton+jets and dilepton final states. In the most sensitive channel (lepton+jets channel), a neural network algorithm that uses lifetime information to identify b-quark jets is used to distinguish signal from background processes. We also present measurements of single top quark production at D0 using several multivariate techniques to separate signal from background.

  13. Critical behavior of cross sections at LHC

    NASA Astrophysics Data System (ADS)

    Dremin, I. M.

    2016-07-01

    Recent experimental data on elastic scattering of high energy protons show that the critical regime has been reached at LHC energies. The approach to criticality is demonstrated by increase of the ratio of elastic to total cross sections from ISR to LHC energies. At LHC it reaches the value which can result in principal change of the character of proton interactions. The treatment of new physics of hollowed toroid-like hadrons requires usage of another branch of the unitarity condition. Its further fate is speculated and interpreted with the help of the unitarity condition in combination with present experimental data. The gedanken experiments to distinguish between different possibilities are proposed.

  14. Neutron absorption cross section of uranium-236

    SciTech Connect

    Macklin, R.L.; Alexander, C.W.

    1988-11-01

    U-236 neutron absorption was measured as a function of neutron time-of-flight from 20 eV to 1 MeV. The neutron flux was monitored with a /sup 6/Li glass scintillator. Average cross sections from 3 keV to 1 MeV were derived. Estimated uncertainties were less than 5% below 600 keV and increased to 9.5% at 1 MeV. Resonance parametrization from 20 eV to a few keV remains to be done. 17 refs., 5 figs., 3 tabs.

  15. Nuclear interaction cross sections for proton radiotherapy

    NASA Astrophysics Data System (ADS)

    Chadwick, M. B.; Jones, D. T. L.; Arendse, G. J.; Cowley, A. A.; Richter, W. A.; Lawrie, J. J.; Newman, R. T.; Pilcher, J. V.; Smit, F. D.; Steyn, G. F.; Koen, JW; Stander, JA

    Model calculations of proton-induced nuclear reaction cross sections are described for biologically-important targets. Measurements made at the National Accelerator Centre are presented for double-differential proton, deuteron, triton, helium-3 and alpha particle spectra, for 150 and 200 MeV protons incident on C, N, and O. These data are needed for Monte Carlo simulations of radiation transport and absorbed dose in proton therapy. Data relevant to the use of positron emission tomography to locate the Bragg peak are also described.

  16. Symmetric charge-transfer cross sections of IIIa rare-earth-metal elements

    SciTech Connect

    Hashida, Masaki; Sakabe, Shuji; Izawa, Yasukazu

    2011-03-15

    Symmetric charge-transfer cross sections of IIIa rare-earth-metal elements (Sc, Y, and Gd) in the impact energy range of 30 to 1000 eV were measured for the first time. The experiments were performed with a crossed-beam apparatus that featured primary ion production by photoionization with a tunable dye laser. Comparing the cross sections of IIIa rare-earth-metal elements ({sigma}{sub Sc}, {sigma}{sub Y}, and {sigma}{sub Gd}) with those of alkali metals or helium {sigma}{sub 0}, we found that {sigma}{sub 0{approx_equal}{sigma}Sc}<{sigma}{sub Y}<{sigma}{sub Gd{approx_equal}}2{sigma}{sub 0}at an impact energy of 1000 eV.

  17. A Congeries of Absorption Cross Sections for Wavelengths Less Than 3000 degrees Angstrom

    NASA Technical Reports Server (NTRS)

    Sullivan, J. O.; Holland, A. C.

    1966-01-01

    The absorption of ultraviolet solar radiation is of prime importance for the study of planetary atmospheres.The absorption coefficients of most of the atmospheric gases have been measured by a number of investigators, but the results are scattered throughout the literature. This report contains a detailed collection of absorption cross sections of the gases listed in Table 1 for wavelengths less than 3000 degrees angstroms. The data on each gas are given together with a historical sketch of the study of the gas and a list of the pertinent references. Also included is a study of the absorption and photoionization coefficients of the major atmospheric gases at intense solar emission lines.

  18. A coupled-cluster study of photodetachment cross sections of closed-shell anions

    SciTech Connect

    Cukras, Janusz; Decleva, Piero; Coriani, Sonia

    2014-11-07

    We investigate the performance of Stieltjes Imaging applied to Lanczos pseudo-spectra generated at the coupled cluster singles and doubles, coupled cluster singles and approximate iterative doubles and coupled cluster singles levels of theory in modeling the photodetachment cross sections of the closed shell anions H{sup −}, Li{sup −}, Na{sup −}, F{sup −}, Cl{sup −}, and OH{sup −}. The accurate description of double excitations is found to play a much more important role than in the case of photoionization of neutral species.

  19. Temperature dependence of the cross section for the fragmentation of thymine via dissociative electron attachment

    SciTech Connect

    Kopyra, Janina; Abdoul-Carime, Hassan

    2015-05-07

    Providing experimental values for absolute Dissociative Electron Attachment (DEA) cross sections for nucleobases at realistic biological conditions is a considerable challenge. In this work, we provide the temperature dependence of the cross section, σ, of the dehydrogenated thymine anion (T − H){sup −} produced via DEA. Within the 393-443 K temperature range, it is observed that σ varies by one order of magnitude. By extrapolating to a temperature of 313 K, the relative DEA cross section for the production of the dehydrogenated thymine anion at an incident energy of 1 eV decreases by 2 orders of magnitude and the absolute value reaches approximately 6 × 10{sup −19} cm{sup 2}. These quantitative measurements provide a benchmark for theoretical prediction and also a contribution to a more accurate description of the effects of ionizing radiation on molecular medium.

  20. Chirality dependence of the absorption cross section of carbon nanotubes.

    PubMed

    Vialla, Fabien; Roquelet, Cyrielle; Langlois, Benjamin; Delport, Géraud; Santos, Silvia Morim; Deleporte, Emmanuelle; Roussignol, Philippe; Delalande, Claude; Voisin, Christophe; Lauret, Jean-Sébastien

    2013-09-27

    The variation of the optical absorption of carbon nanotubes with their geometry has been a long-standing question at the heart of both metrological and applicative issues, in particular because optical spectroscopy is one of the primary tools for the assessment of the chiral species abundance of samples. Here, we tackle the chirality dependence of the optical absorption with an original method involving ultraefficient energy transfer in porphyrin-nanotube compounds that allows uniform photoexcitation of all chiral species. We measure the absolute absorption cross section of a wide range of semiconducting nanotubes at their S22 transition and show that it varies by up to a factor of 2.2 with the chiral angle, with type I nanotubes showing a larger absorption. In contrast, the luminescence quantum yield remains almost constant.

  1. Chirality Dependence of the Absorption Cross Section of Carbon Nanotubes

    NASA Astrophysics Data System (ADS)

    Vialla, Fabien; Roquelet, Cyrielle; Langlois, Benjamin; Delport, Géraud; Santos, Silvia Morim; Deleporte, Emmanuelle; Roussignol, Philippe; Delalande, Claude; Voisin, Christophe; Lauret, Jean-Sébastien

    2013-09-01

    The variation of the optical absorption of carbon nanotubes with their geometry has been a long-standing question at the heart of both metrological and applicative issues, in particular because optical spectroscopy is one of the primary tools for the assessment of the chiral species abundance of samples. Here, we tackle the chirality dependence of the optical absorption with an original method involving ultraefficient energy transfer in porphyrin-nanotube compounds that allows uniform photoexcitation of all chiral species. We measure the absolute absorption cross section of a wide range of semiconducting nanotubes at their S22 transition and show that it varies by up to a factor of 2.2 with the chiral angle, with type I nanotubes showing a larger absorption. In contrast, the luminescence quantum yield remains almost constant.

  2. Photoionization and photofragmentation of the C60+ molecular ion

    SciTech Connect

    Baral, K. K.; Aryal, N. B.; Esteves-Macaluso, D. A.; Thomas, C. M.; Hellhund, J.; Lomsadze, R.; Kilcoyne, A. L. D.; Müller, A.; Schippers, S.; Phaneuf, R. A.

    2016-03-01

    Cross-section measurements are reported for single and double photoionization of C$+\\atop{60}$ ions in the photon energy range 18-150 eV accompanied by the loss of zero to seven pairs of carbon atoms, as well as for fragmentation without ionization resulting in loss of two to eight pairs of C atoms in the photon energy range 18-65 eV. Absolute measurements were performed by merging a beam of C$+\\atop{60}$ molecular ions with a beam of monochromatized synchrotron radiation. Product channels involving dissociation yielding smaller fullerene fragment ions account for nearly half of the total measured oscillator strength in this energy range. The sum of cross sections for the measured product channels is compared to a published calculation of the total photoabsorption cross section of neutral C60 based on time-dependent density-functional theory. Lastly, this comparison and an accounting of oscillator strengths indicate that with the exception of C$+\\atop{58}$, the most important product channels resulting from photoabsorption were accounted for in the experiment. Threshold energies for the successive removal of carbon atom pairs accompanying photoionization are also determined from the measurements.

  3. Positronium beam production and scattering cross-sections

    NASA Astrophysics Data System (ADS)

    Leslie, Dawn Elizabeth

    In this work, the efficiency for the production of a monoenergetic positronium beam via the charge-exchange reaction of a positron beam in a gaseous target has been determined for molecular hydrogen and molecular nitrogen. In the case of molecular nitrogen, it has been found that the energy range over which a useful intensity of collimated positronium may be produced can be extended to 250eV, 100eV higher than previously achieved. This should enable measurements of the total and partial positronium cross-sections at correspondingly higher energies, where target inelastic effects are expected to be significant A recent measurement of the integrated positronium formation cross-section for xenon found a larger yield of positronium atoms compared to the other noble gases. A shoulder was also seen 10eV above the peak and it was suggested that this might be due to the production of positronium in an excited state. These findings have provided an incentive to investigate the collimated positronium production efficiency from xenon, which has been found to be surprisingly low. The quantum state of the beam atoms has also been found to be dominantly ground state. Possible reasons for these findings are discussed Total cross-sections for positronium-gas scattering have been extracted from the measurements of the positronium beam production efficiency for both molecular nitrogen and xenon. These quantities have also been determined directly by measuring the intensity of the positronium beam transmitted through a gas cell via the Beer-Lambert Law. A good consistency is found between the values obtained using this method and those determined indirectly. Recently, measurements have been made of the absolute integrated cross-section for the fragmentation of positronium in collision with helium atoms, along with the longitudinal energy distributions of the residual positrons in the energy range -Ep/=13-33eV. Measurements of the latter indicate a peak close to half the residual

  4. Pion production cross sections and associated parameters

    NASA Astrophysics Data System (ADS)

    Bradbury, J. N.

    Negative pions have been used for radiotherapy at the meson factories LAMPF (USA), SIN (Switzerland), and TRIUMF (Canada) and have been planned for use at new meson facilities under construction (USSR) and at proposed dedicated medical facilities. Providing therapeutically useful dose rates of pions requires a knowledge of the pion production cross sections as a function of primary proton energy (500 to 1000 MeV), pion energy (less than or equal to100 MeV), production angle, and target material. The current status of the data base in this area is presented including theoretical guidelines for extrapolation purposes. The target material and geometry, as well as the proton and pion beam parameters, will affect the electron (and muon) contamination in the beam which may have an important effect on both the LET characteristics of the dose and the dose distribution. In addition to cross-section data, channel characteristics such as length of pion trajectory, solid-angle acceptance, and momentum analysis will affect dose rate, distribution, and quality. Such considerations are briefly addressed in terms of existing facilities and proposed systems.

  5. Total cross sections for neutron scattering

    NASA Astrophysics Data System (ADS)

    Chinn, C. R.; Elster, Ch.; Thaler, R. M.; Weppner, S. P.

    1995-02-01

    Measurements of neutron total cross sections are both extensive and extremely accurate. Although they place a strong constraint on theoretically constructed models, there are relatively few comparisons of predictions with experiment. The total cross sections for neutron scattering from 16O and 40Ca are calculated as a function of energy from 50 to 700 MeV laboratory energy with a microscopic first-order optical potential derived within the framework of the Watson expansion. Although these results are aleady in qualitative agreement with the data, the inclusion of medium corrections to the propagator is essential to correctly predict the energy dependence given by the experiment. In the region between 100 and 200 MeV, where off-shell tρ calculations for both 16O and 40Ca overpredict the experiment, the modification due to the nuclear medium reduces the calculated values. Above 300 MeV these corrections are very small and depending on the employed nuclear mean field tend to compensate for the underprediction of the off-shell tρ results.

  6. Classical calculation of ionization and electron-capture total cross sections in H{sup +}+H{sub 2}O collisions

    SciTech Connect

    Errea, L. F.; Illescas, Clara; Mendez, L.; Rabadan, I.; Riera, A.; Pons, B.

    2007-10-15

    We report total cross sections for single ionization and electron capture in H{sup +} collisions with water molecules at impact energies 25 keVcross sections by multiplying the partial cross sections by the branching ratios measured in the photoionization experiments of Tan et al. [Chem. Phys. Lett. 29, 299 (1978)].

  7. Calculations of photo-induced X-ray production cross-sections in the energy range 1-150 keV and average fluorescence yields for Zn, Cd and Hg

    NASA Astrophysics Data System (ADS)

    Sampaio, J. M.; Guerra, M.; Parente, F.; Madeira, T. I.; Indelicato, P.; Santos, J. P.; Marques, J. P.

    2016-09-01

    In this paper, we calculate the K-, L- and M-shells X-ray production, and X-ray fluorescence cross-sections after photo-induced ionization, for Zn, Cd, and Hg, and for incident photon energy range from 1 to 150 keV. For this purpose, the corresponding average fluorescence yields for Zn, Cd, and Hg as well as the photoionization cross-sections were calculated using the Dirac-Fock method. Subshell fluorescence, intrashell and intershell yields are obtained consistently from radiative and radiationless transitions calculated in the exact same method. A comprehensive account of the relations between the X-ray production, X-ray fluorescence cross-sections and the photoionization cross-sections and these yields is presented. Comparisons are made with results from other authors. The obtained values for the photoionization cross-sections are in good agreement with the widely used data of Scofield in the studied energy range. However our results for the X-ray fluorescence cross sections seem to favor some data relatively to others. The energy dependence of the average fluorescence yields is discussed, in particular, the reliability of extrapolated data for lighter elements from measurements and calculations in heavier elements above the inner shell absorption edges is questioned. Tabulated data on photoionization and X-ray production cross-sections are presented for the incident photon energy range 1-150 keV in steps of 1 keV.

  8. Accurate universal parameterization of absorption cross sections II--neutron absorption cross sections

    NASA Technical Reports Server (NTRS)

    Tripathi, R. K.; Wilson, J. W.; Cucinotta, F. A.

    1997-01-01

    A recent parameterization (here after referred as paper I, Ref. [4]) of absorption cross sections for any system of charged ions collisions including proton -nucleus collisions, is extended for neutron-nucleus collisions valid from approximately 1 MeV to a few GeV, thus providing a comprehensive picture of absorption cross sections for any system of collision pair (charged and/or uncharged). The parameters are associated with the physics of the problem. At lower energies, the optical potential at the surface is important and the Pauli operator plays an increasingly important role at intermediate energies. The agreement between the calculated and experimental data is better than earlier published results.

  9. Accurate universal parameterization of absorption cross sections II — neutron absorption cross sections

    NASA Astrophysics Data System (ADS)

    Tripathi, R. K.; Wilson, John W.; Cucinotta, Francis A.

    1997-06-01

    A recent parameterization (here after referred as paper I, Ref. [4]) of absorption cross sections for any system of charged ions collisions including proton -nucleus collisions, is extended for neutron-nucleus collisions valid from ˜ 1 MeV to a few GeV, thus providing a comprehensive picture of absorption cross sections for any system of collision pair (charged and/or uncharged). The parameters are associated with the physics of the problem. At lower energies, the optical potential at the surface is important and the Pauli operator plays an increasingly important role at intermediate energies. The agreement between the calculated and experimental data is better than earlier published results.

  10. Helium 23S photoionization up to the N = 5 threshold

    NASA Astrophysics Data System (ADS)

    Argenti, Luca; Moccia, Roberto

    2008-02-01

    We present the results of an accurate B-spline K-matrix calculation of total and partial cross sections and asymmetry parameters for the photoionization of the metastable 23Se state of helium up to the N = 5 threshold. The effect of the [040]+5 intruder state below N = 4 is shown.

  11. Geophysical Fluid Flow Cell (GFFC) Cross Section

    NASA Technical Reports Server (NTRS)

    1995-01-01

    This drawing shows a cross-section view of the test cell at the heart of the Geophysical Fluid Flow Cell (GFFC) that flew on two Spacelab missions. The middle and lower drawings depict the volume of the silicone oil layer that served as the atmosphere as the steel ball rotated and an electrostatic field pulled the oil inward to mimic gravity's effects during the experiments. The GFFC thus produced flow patterns that simulated conditions inside the atmospheres of Jupiter and the Sun and other stars. The principal investigator was John Hart of the University of Colorado at Boulder. It was managed by NASA's Marshall Space Flight Center (MSFC). An Acrobat PDF copy of this drawing is available at http://microgravity.nasa.gov/gallery. (Credit: NASA/Marshall Space Flight Center)

  12. Neutrino Cross Sections at Supernova Energies

    NASA Astrophysics Data System (ADS)

    Scholberg, Kate

    2017-01-01

    Neutrinos with energies between a few and a few tens of MeV are relevant for a number of physics topics. Notably, this is the energy range corresponding to emission of neutrinos from supernovae. In addition, it is relevant for studies of solar, reactor and atmospheric neutrinos, as well as for physics using accelerator-produced neutrinos from pions or radioactive nuclei decaying at rest. Surprisingly, with the exception of interactions on electrons and protons, the interactions of neutrinos with matter in this energy range are quite poorly understood, both theoretically and experimentally. This talk will describe neutrino physics and astrophysics in the supernova-neutrino energy range, the state of knowledge of cross sections on relevant nuclei, and initiatives for experimental measurements.

  13. Lunar Radar Cross Section at Low Frequency

    NASA Technical Reports Server (NTRS)

    Rodriguez, P.; Kennedy, E. J.; Kossey, P.; McCarrick, M.; Kaiser, M. L.; Bougeret, J.-L.; Tokarev, Y. V.

    2002-01-01

    Recent bistatic measurements of the lunar radar cross-section have extended the spectrum to long radio wavelength. We have utilized the HF Active Auroral Research Program (HAARP) radar facility near Gakona, Alaska to transmit high power pulses at 8.075 MHz to the Moon; the echo pulses were received onboard the NASA/WIND spacecraft by the WAVES HF receiver. This lunar radar experiment follows our previous use of earth-based HF radar with satellites to conduct space experiments. The spacecraft was approaching the Moon for a scheduled orbit perturbation when our experiment of 13 September 2001 was conducted. During the two-hour experiment, the radial distance of the satellite from the Moon varied from 28 to 24 Rm, where Rm is in lunar radii.

  14. Top cross section measurement at CDF

    SciTech Connect

    Compostella, Gabriele; /INFN, CNAF /Padua U.

    2010-01-01

    This paper describes the latest measurements of the t{bar t} pair production cross section performed by the CDF Collaboration analyzing p{bar p} collisions at a center-of-mass energy of 1.96 TeV from Fermilab Tevatron, as presented at the XVIII International Workshop on Deep-Inelastic Scattering and Related Subjects. In order to test Standard Model predictions, several analysis methods are explored and all the top decay channels are considered, to better constrain the properties of the top quark and to search for possible sources of new physics affecting the pair production mechanism. Experimental results using an integrated luminosity up to 5.1 fb{sup -1} are presented.

  15. Angle-averaged Compton cross sections

    SciTech Connect

    Nickel, G.H.

    1983-01-01

    The scattering of a photon by an individual free electron is characterized by six quantities: ..cap alpha.. = initial photon energy in units of m/sub 0/c/sup 2/; ..cap alpha../sub s/ = scattered photon energy in units of m/sub 0/c/sup 2/; ..beta.. = initial electron velocity in units of c; phi = angle between photon direction and electron direction in the laboratory frame (LF); theta = polar angle change due to Compton scattering, measured in the electron rest frame (ERF); and tau = azimuthal angle change in the ERF. We present an analytic expression for the average of the Compton cross section over phi, theta, and tau. The lowest order approximation to this equation is reasonably accurate for photons and electrons with energies of many keV.

  16. Preliminary cross section of Englebright Lake sediments

    USGS Publications Warehouse

    Snyder, Noah P.; Hampton, Margaret A.

    2003-01-01

    Overview -- The Upper Yuba River Studies Program is a CALFED-funded, multidisciplinary investigation of the feasibility of introducing anadromous fish species to the Yuba River system upstream of Englebright Dam. Englebright Lake (Figure 1 on poster) is a narrow, 14-km-long reservoir located in the northern Sierra Nevada, northeast of Marysville, CA. The dam was completed in 1941 for the primary purpose of trapping sediment derived from mining operations in the Yuba River watershed. Possible management scenarios include lowering or removing Englebright Dam, which could cause the release of stored sediments and associated contaminants, such as mercury used extensively in 19th-century hydraulic gold mining. Transport of released sediment to downstream areas could increase existing problems including flooding and mercury bioaccumulation in sport fish. To characterize the extent, grain size, and chemistry of this sediment, a coring campaign was done in Englebright Lake in May and June 2002. More than twenty holes were drilled at 7 different locations along the longitudinal axis of the reservoir (Figure 4 on poster), recovering 6 complete sequences of post-reservoir deposition and progradation. Here, a longitudinal cross section of Englebright Lake is presented (Figure 5 on poster), including pre-dam and present-day topographic profiles, and sedimentologic sections for each coring site. This figure shows the deltaic form of the reservoir deposit, with a thick upper section consisting of sand and gravel overlying silt, a steep front, and a thinner lower section dominated by silt. The methodologies used to create the reservoir cross section are discussed in the lower part of this poster.

  17. Measurements of the Ultraviolet Fluorescence Cross Sections and Spectra of Bacillus Anthracis Simulants

    SciTech Connect

    Stephens, J.R.

    1998-09-01

    Measurements of the ultraviolet autofluorescence spectra and absolute cross sections of the Bacillus anthracis (Ba) simulants Bacillus globigii (Bg), Bacillus megaterium (Bm), Bacillus subtilis (Bs), and Bacillus cereus (Bc) were measured. Fluorescence spectra and cross sections of pine pollen (Pina echinata) were measured for comparison. Both dried vegetative cells and spores separated from the sporulated vegetative material were studied. The spectra were obtained by suspending a small number (<10) of particles in air in our Single Particle Spectroscopy Apparatus (SPSA), illuminating the particles with light from a spectrally filtered arc lamp, and measuring the fluorescence spectra of the particles. The illumination was 280 nm (20 nm FWHM) and the fluorescence spectra was measured between 300 and 450 nm. The fluorescence cross section of vegetative Bg peaks at 320 nm with a maximum cross section of 5 X 10{sup -14} cm{sup 2}/sr-nm-particle while the Bg spore fluorescence peaks at 310 nm with peak fluorescence of 8 X 10{sup -15} cm{sup 2}/sr-nm-particle. Pine pollen particles showed a higher fluorescence peaking at 355 nm with a cross section of 1.7 X 10{sup -13} cm{sup 2}/sr-nm-particle. Integrated cross sections ranged from 3.0 X 10{sup -13} for the Bg spores through 2.25 X 10{sup -12} (cm{sup 2}/sr-particle) for the vegetative cells.

  18. Status update on the NIFFTE high precision fission cross section measurement program

    SciTech Connect

    Laptev, Alexander B; Tovesson, Fredrik; Burgett, Eric; Greife, Uwe; Grimes, Steven; Heffner, Michael D; Hertel, Nolan E; Hill, Tony; Isenhower, Donald; Klay, Jennifer L; Kornilov, Nickolay; Kudo, Ryuho; Loveland, Walter; Massey, Thomas; Mc Grath, Chris; Pickle, Nathan; Qu, Hai; Sharma, Sarvagya; Snyder, Lucas; Thornton, Tyler; Towell, Rusty S; Watson, Shon

    2010-01-01

    The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) program has been underway for nearly two years. The program's mission is to measure fission cross sections of the primary fissionable and fissile materials ({sup 235}U, {sup 239}Pu, {sup 238}U) as well as the minor actinides across energies from approximately 50 keV up to 20 MeV with an absolute uncertainty of less than one percent while investigating energy ranges from below an eV to 600 MeV. This basic nuclear physics data is being reinvestigated to support the next generation power plants and a fast burner reactor program. Uncertainties in the fast, resolved and unresolved resonance regions in plutonium and other transuranics are extremely large, dominating safety margins in the next generation nuclear power plants and power plants of today. This basic nuclear data can be used to support all aspects of the nuciear renaissance. The measurement campaign is utilizing a Time Projection Chamber or TPC as the tool to measure these cross sections to these unprecedented levels. Unlike traditional fission cross section measurements using time-of-flight and a multiple fission foil configurations in which fission cross sections in relation to that of {sup 235}U are performed, the TPC project uses time-of-flight and hydrogen as the benchmark cross section. Using the switch to hydrogen, a simple, smooth cross section that can be used which removes the uncertainties associated with the resolved and unresolved resonances in {sup 235}U.

  19. Single-level resonance parameters fit nuclear cross-sections

    NASA Technical Reports Server (NTRS)

    Drawbaugh, D. W.; Gibson, G.; Miller, M.; Page, S. L.

    1970-01-01

    Least squares analyses of experimental differential cross-section data for the U-235 nucleus have yielded single level Breit-Wigner resonance parameters that fit, simultaneously, three nuclear cross sections of capture, fission, and total.

  20. Experiments on Antiprotons: Antiproton-Nucleon Cross Sections

    DOE R&D Accomplishments Database

    Chamberlain, Owen; Keller, Donald V.; Mermond, Ronald; Segre, Emilio; Steiner, Herbert M.; Ypsilantis, Tom

    1957-07-22

    In this paper experiments are reported on annihilation and scattering of antiprotons in H{sub 2}O , D{sub 2}O, and O{sub 2}. From the data measured it is possible to obtain an antiproton-proton and an antiproton-deuteron cross section at 457 Mev (lab). Further analysis gives the p-p and p-n cross sections as 104 mb for the p-p reaction cross section and 113 mb for the p-n reaction cross section. The respective annihilation cross sections are 89 and 74 mb. The Glauber correction necessary in order to pass from the p-d to the p-n cross section by subtraction of the p-p cross section is unfortunately large and somewhat uncertain. The data are compared with the p-p and p-n cross sections and with other results on p-p collisions.

  1. Total and ionization cross sections of electron scattering by fluorocarbons

    NASA Astrophysics Data System (ADS)

    Antony, B. K.; Joshipura, K. N.; Mason, N. J.

    2005-02-01

    Electron impact total cross sections (50-2000 eV) and total ionization cross sections (threshold to 2000 eV) are calculated for typical plasma etching molecules CF4, C2F4, C2F6, C3F8 and CF3I and the CFx (x = 1-3) radicals. The total elastic and inelastic cross sections are determined in the spherical complex potential formalism. The sum of the two gives the total cross section and the total inelastic cross section is used to calculate the total ionization cross sections. The present total and ionization cross sections are found to be consistent with other theories and experimental measurements, where they exist. Our total cross section results for CFx (x = 1-3) radicals presented here are first estimates on these species.

  2. Collision Cross Sections for 20 Protonated Amino Acids: Fourier Transform Ion Cyclotron Resonance and Ion Mobility Results

    NASA Astrophysics Data System (ADS)

    Anupriya; Jones, Chad A.; Dearden, David V.

    2016-08-01

    We report relative dephasing cross sections for the 20 biogenic protonated amino acids measured using the cross sectional areas by Fourier transform ion cyclotron resonance (CRAFTI) technique at 1.9 keV in the laboratory reference frame, as well as momentum transfer cross sections for the same ions computed from Boltzmann-weighted structures determined using molecular mechanics. Cross sections generally increase with increasing molecular weight. Cross sections for aliphatic and aromatic protonated amino acids are larger than the average trend, suggesting these side chains do not fold efficiently. Sulfur-containing protonated amino acids have smaller than average cross sections, reflecting the mass of the S atom. Protonated amino acids that can internally hydrogen-bond have smaller than average cross sections, reflecting more extensive folding. The CRAFTI measurements correlate well with results from drift ion mobility (IMS) and traveling wave ion mobility (TWIMS) spectrometric measurements; CRAFTI results correlate with IMS values approximately as well as IMS and TWIMS values from independent measurements correlate with each other. Both CRAFTI and IMS results correlate well with the computed momentum transfer cross sections, suggesting both techniques provide accurate molecular structural information. Absolute values obtained using the various methods differ significantly; in the case of CRAFTI, this may be due to errors in measurements of collision gas pressure, measurement of excitation voltage, and/or dependence of cross sections on kinetic energy.

  3. Electron Elastic-Scattering Cross-Section Database

    National Institute of Standards and Technology Data Gateway

    SRD 64 NIST Electron Elastic-Scattering Cross-Section Database (PC database, no charge)   This database provides values of differential elastic-scattering cross sections, corresponding total elastic-scattering cross sections, phase shifts, and transport cross sections for elements with atomic numbers from 1 to 96 and for electron energies between 50 eV and 20,000 eV (in steps of 1 eV).

  4. Mental Visualization of Objects from Cross-Sectional Images

    ERIC Educational Resources Information Center

    Wu, Bing; Klatzky, Roberta L.; Stetten, George D.

    2012-01-01

    We extended the classic anorthoscopic viewing procedure to test a model of visualization of 3D structures from 2D cross-sections. Four experiments were conducted to examine key processes described in the model, localizing cross-sections within a common frame of reference and spatiotemporal integration of cross sections into a hierarchical object…

  5. Inclusive Neutrino Cross Section Measurements at MINERvA

    NASA Astrophysics Data System (ADS)

    Tice, Brian

    2012-10-01

    MINERvA part 4. The knowledge of inclusive neutrino cross sections is valuable for neutrino oscillation experiments. Determination of the A dependence of the cross section can help determine the role of nuclear effects in neutrino scattering, which is poorly known and difficult to model. Preliminary ratios of cross sections on carbon, iron and lead will be shown.

  6. Mental Visualization of Objects from Cross-Sectional Images

    ERIC Educational Resources Information Center

    Wu, Bing; Klatzky, Roberta L.; Stetten, George D.

    2012-01-01

    We extended the classic anorthoscopic viewing procedure to test a model of visualization of 3D structures from 2D cross-sections. Four experiments were conducted to examine key processes described in the model, localizing cross-sections within a common frame of reference and spatiotemporal integration of cross sections into a hierarchical object…

  7. Viscous Flow through Pipes of Various Cross-Sections

    ERIC Educational Resources Information Center

    Lekner, John

    2007-01-01

    An interesting variety of pipe cross-sectional shapes can be generated, for which the Navier-Stokes equations can be solved exactly. The simplest cases include the known solutions for elliptical and equilateral triangle cross-sections. Students can find pipe cross-sections from solutions of Laplace's equation in two dimensions, and then plot the…

  8. Ratio of Jet Cross Sections at s = 630 GeV and 1800 GeV

    NASA Astrophysics Data System (ADS)

    Abbott, B.; Abolins, M.; Abramov, V.; Acharya, B. S.; Adams, D. L.; Adams, M.; Alves, G. A.; Amos, N.; Anderson, E. W.; Baarmand, M. M.; Babintsev, V. V.; Babukhadia, L.; Baden, A.; Baldin, B.; Balm, P. W.; Banerjee, S.; Bantly, J.; Barberis, E.; Baringer, P.; Bartlett, J. F.; Bassler, U.; Bean, A.; Begel, M.; Belyaev, A.; Beri, S. B.; Bernardi, G.; Bertram, I.; Besson, A.; Bezzubov, V. A.; Bhat, P. C.; Bhatnagar, V.; Bhattacharjee, M.; Blazey, G.; Blessing, S.; Boehnlein, A.; Bojko, N. I.; Borcherding, F.; Brandt, A.; Breedon, R.; Briskin, G.; Brock, R.; Brooijmans, G.; Bross, A.; Buchholz, D.; Buehler, M.; Buescher, V.; Burtovoi, V. S.; Butler, J. M.; Canelli, F.; Carvalho, W.; Casey, D.; Casilum, Z.; Castilla-Valdez, H.; Chakraborty, D.; Chan, K. M.; Chekulaev, S. V.; Cho, D. K.; Choi, S.; Chopra, S.; Christenson, J. H.; Chung, M.; Claes, D.; Clark, A. R.; Cochran, J.; Coney, L.; Connolly, B.; Cooper, W. E.; Coppage, D.; Cummings, M. A.; Cutts, D.; Dahl, O. I.; Davis, G. A.; Davis, K.; de, K.; del Signore, K.; Demarteau, M.; Demina, R.; Demine, P.; Denisov, D.; Denisov, S. P.; Desai, S.; Diehl, H. T.; Diesburg, M.; di Loreto, G.; Doulas, S.; Draper, P.; Ducros, Y.; Dudko, L. V.; Duensing, S.; Dugad, S. R.; Dyshkant, A.; Edmunds, D.; Ellison, J.; Elvira, V. D.; Engelmann, R.; Eno, S.; Eppley, G.; Ermolov, P.; Eroshin, O. V.; Estrada, J.; Evans, H.; Evdokimov, V. N.; Fahland, T.; Feher, S.; Fein, D.; Ferbel, T.; Fisk, H. E.; Fisyak, Y.; Flattum, E.; Fleuret, F.; Fortner, M.; Frame, K. C.; Fuess, S.; Gallas, E.; Galyaev, A. N.; Gartung, P.; Gavrilov, V.; Genik, R. J.; Genser, K.; Gerber, C. E.; Gershtein, Y.; Gibbard, B.; Gilmartin, R.; Ginther, G.; Gómez, B.; Gómez, G.; Goncharov, P. I.; González Solís, J. L.; Gordon, H.; Goss, L. T.; Gounder, K.; Goussiou, A.; Graf, N.; Graham, G.; Grannis, P. D.; Green, J. A.; Greenlee, H.; Grinstein, S.; Groer, L.; Grudberg, P.; Grünendahl, S.; Gupta, A.; Gurzhiev, S. N.; Gutierrez, G.; Gutierrez, P.; Hadley, N. J.; Haggerty, H.; Hagopian, S.; Hagopian, V.; Hahn, K. S.; Hall, R. E.; Hanlet, P.; Hansen, S.; Hauptman, J. M.; Hays, C.; Hebert, C.; Hedin, D.; Heinson, A. P.; Heintz, U.; Heuring, T.; Hirosky, R.; Hobbs, J. D.; Hoeneisen, B.; Hoftun, J. S.; Hou, S.; Huang, Y.; Ito, A. S.; Jerger, S. A.; Jesik, R.; Johns, K.; Johnson, M.; Jonckheere, A.; Jones, M.; Jöstlein, H.; Juste, A.; Kahn, S.; Kajfasz, E.; Karmanov, D.; Karmgard, D.; Kehoe, R.; Kim, S. K.; Klima, B.; Klopfenstein, C.; Knuteson, B.; Ko, W.; Kohli, J. M.; Kostritskiy, A. V.; Kotcher, J.; Kotwal, A. V.; Kozelov, A. V.; Kozlovsky, E. A.; Krane, J.; Krishnaswamy, M. R.; Krzywdzinski, S.; Kubantsev, M.; Kuleshov, S.; Kulik, Y.; Kunori, S.; Kuznetsov, V. E.; Landsberg, G.; Leflat, A.; Lehner, F.; Li, J.; Li, Q. Z.; Lima, J. G.; Lincoln, D.; Linn, S. L.; Linnemann, J.; Lipton, R.; Lucotte, A.; Lueking, L.; Lundstedt, C.; Maciel, A. K.; Madaras, R. J.; Manankov, V.; Mao, H. S.; Marshall, T.; Martin, M. I.; Martin, R. D.; Mauritz, K. M.; May, B.; Mayorov, A. A.; McCarthy, R.; McDonald, J.; McMahon, T.; Melanson, H. L.; Meng, X. C.; Merkin, M.; Merritt, K. W.; Miao, C.; Miettinen, H.; Mihalcea, D.; Mincer, A.; Mishra, C. S.; Mokhov, N.; Mondal, N. K.; Montgomery, H. E.; Moore, R. W.; Mostafa, M.; da Motta, H.; Nagy, E.; Nang, F.; Narain, M.; Narasimham, V. S.; Neal, H. A.; Negret, J. P.; Negroni, S.; Norman, D.; Oesch, L.; Oguri, V.; Olivier, B.; Oshima, N.; Padley, P.; Pan, L. J.; Para, A.; Parashar, N.; Partridge, R.; Parua, N.; Paterno, M.; Patwa, A.; Pawlik, B.; Perkins, J.; Peters, M.; Peters, O.; Piegaia, R.; Piekarz, H.; Pope, B. G.; Popkov, E.; Prosper, H. B.; Protopopescu, S.; Qian, J.; Quintas, P. Z.; Raja, R.; Rajagopalan, S.; Ramberg, E.; Rapidis, P. A.; Reay, N. W.; Reucroft, S.; Rha, J.; Rijssenbeek, M.; Rockwell, T.; Roco, M.; Rubinov, P.; Ruchti, R.; Rutherfoord, J.; Santoro, A.; Sawyer, L.; Schamberger, R. D.; Schellman, H.; Schwartzman, A.; Sculli, J.; Sen, N.; Shabalina, E.; Shankar, H. C.; Shivpuri, R. K.; Shpakov, D.; Shupe, M.; Sidwell, R. A.; Simak, V.; Singh, H.; Singh, J. B.; Sirotenko, V.; Slattery, P.; Smith, E.; Smith, R. P.; Snihur, R.; Snow, G. R.; Snow, J.; Snyder, S.; Solomon, J.; Sorín, V.; Sosebee, M.; Sotnikova, N.; Soustruznik, K.; Souza, M.; Stanton, N. R.; Steinbrück, G.; Stephens, R. W.; Stevenson, M. L.; Stichelbaut, F.; Stoker, D.; Stolin, V.; Stoyanova, D. A.; Strauss, M.; Streets, K.; Strovink, M.; Stutte, L.; Sznajder, A.; Taylor, W.; Tentindo-Repond, S.; Thompson, J.; Toback, D.; Tripathi, S. M.; Trippe, T. G.; Turcot, A. S.; Tuts, P. M.; van Gemmeren, P.; Vaniev, V.; van Kooten, R.; Varelas, N.; Volkov, A. A.; Vorobiev, A. P.; Wahl, H. D.; Wang, H.; Wang, Z.-M.; Warchol, J.; Watts, G.; Wayne, M.; Weerts, H.; White, A.; White, J. T.; Whiteson, D.; Wightman, J. A.; Wijngaarden, D. A.; Willis, S.; Wimpenny, S. J.; Wirjawan, J. V.; Womersley, J.; Wood, D. R.; Yamada, R.; Yamin, P.; Yasuda, T.; Yip, K.; Youssef, S.; Yu, J.; Yu, Z.; Zanabria, M.; Zheng, H.; Zhou, Z.; Zhu, Z. H.; Zielinski, M.; Zieminska, D.; Zieminski, A.; Zutshi, V.; Zverev, E. G.; Zylberstejn, A.

    2001-03-01

    The D0 Collaboration has measured the inclusive jet cross section in p¯p collisions at s = 630 GeV. The results for pseudorapidities η<0.5 are combined with our previous results at s = 1800 GeV to form a ratio of cross sections with smaller uncertainties than either individual measurement. Next-to-leading-order QCD predictions show excellent agreement with the measurement at 630 GeV; agreement is also satisfactory for the ratio. Specifically, despite a 10% to 15% difference in the absolute magnitude, the dependence of the ratio on jet transverse momentum is very similar for data and theory.

  9. Integral cross sections for π+p interactions at low energies

    NASA Astrophysics Data System (ADS)

    Friedman, E.; Goldring, A.; Wagner, G. J.; Altman, A.; Johnson, R. R.; Meirav, O.; Jennings, B. K.

    1990-08-01

    Integral cross sections for the elastic scattering of π+ by protons into angles greater than 20° or 30° (lab) have been measured by the beam-attenuation technique over the energy range of 45-126MeV. The measurements are aimed at providing independent checks on the absolute normalization of differential cross sections, where discrepancies exist between different data sets. Comparisons with predictions made with existing phase shifts show very good agreement with the dispersion-relation constrained phase shifts of the Karlsruhe group.

  10. Photoionization of ground and excited levels of P II

    NASA Astrophysics Data System (ADS)

    Nahar, Sultana N.

    2017-01-01

    Photoionization cross section (σPI) of P II, (hν + P II → P III + e), from ground and a large number of excited levels are presented. The study includes the resonant structures and the characteristics of the background in photoionization cross sections. The present calculations were carried out in the Breit-Pauli R-matrix (BPRM) method that includes relativistic effects. The autoionizing resonances are delineated with a fine energy mesh to observe the fine structure effects. A singular resonance, formed by the coupling of channels in fine structure but not allowed in LS coupling, is seen at the ionization threshold of photoionization for the ground and many excited levels. The background cross section is seen enhanced compared to smooth decay for the excited levels. Examples are presented to illustrate the enhanced background cross sections at the energies of the core levels, 4P3/2 and 2D3/2, that are allowed for electric dipole transitions by the core ground level 2 P1/2o. In addition strong Seaton or photo-excitation-of-core (PEC) resonances are found in the photoionization of single valence electron excited levels. Calculations used a close coupling wave function expansion that included 18 fine structure levels of core P III from configurations 3s23p, 3s3p2, 3s23d, 3s24s, 3s24p and 3p3. Photoionization cross sections are presented for all 475 fine structure levels of P II found with n ≤ 10 and l ≤ 9. The present results will provide high precision parameters of various applications involving this less studied ion.

  11. s-wave threshold in electron attachment - Observations and cross sections in CCl4 and SF6 at ultralow electron energies

    NASA Technical Reports Server (NTRS)

    Chutjian, A.; Alajajian, S. H.

    1985-01-01

    The threshold photoionization method was used to study low-energy electron attachment phenomena in and cross sections of CCl4 and SF6 compounds, which have applications in the design of gaseous dielectrics and diffuse discharge opening switches. Measurements were made at electron energies from below threshold to 140 meV at resolutions of 6 and 8 meV. A narrow resolution-limited structure was observed in electron attachment to CCl4 and SF6 at electron energies below 10 meV, which is attributed to the divergence of the attachment cross section in the limit epsilon, l approaches zero. The results are compared with experimental collisional-ionization results, electron-swarm unfolded cross sections, and earlier threshold photoionization data.

  12. s-wave threshold in electron attachment - Observations and cross sections in CCl4 and SF6 at ultralow electron energies

    NASA Technical Reports Server (NTRS)

    Chutjian, A.; Alajajian, S. H.

    1985-01-01

    The threshold photoionization method was used to study low-energy electron attachment phenomena in and cross sections of CCl4 and SF6 compounds, which have applications in the design of gaseous dielectrics and diffuse discharge opening switches. Measurements were made at electron energies from below threshold to 140 meV at resolutions of 6 and 8 meV. A narrow resolution-limited structure was observed in electron attachment to CCl4 and SF6 at electron energies below 10 meV, which is attributed to the divergence of the attachment cross section in the limit epsilon, l approaches zero. The results are compared with experimental collisional-ionization results, electron-swarm unfolded cross sections, and earlier threshold photoionization data.

  13. Current distribution in ESD diodes; Cross section corrections

    NASA Astrophysics Data System (ADS)

    Lin, J. C.; Gomer, R.

    1986-06-01

    The electron current distribution in diodes consisting of a rectangular crystal and an electron emitting filament parallel to and in front of it, used in several electron stimulated desorption (ESD) experiments has been determined by means of a dummy crystal constructed from uniformly transparent Lektromesh and a moveable, suitably constructed fine probe. It was found that for straight filaments the distribution was uniform along the narrow, but nearly triangular along the long dimension of the crystal. Calculated log signal versus time curves in ESD show considerable curvature, as often observed experimentally with such geometries. Filaments with a straight center, but coiled and shielded end sections provide uniform current distributions. When such filaments are used the curvature of the log signal versus time curves disappears for Kr desorption from W(110) but is still seen for oxygen desorption. The absolute fraction of filament current hitting the front surface of a crystal was also determined for various geometries by using a thin suppressor mesh in front of the dummy crystal. Cross sections for CO, O, and Kr ESD from W(110) were redetermined with a coiled end section filament. After correction for the fractions of current to the crystal and current non-uniformities previous results are in fairly reasonable agreement with the new values, except for the CO measurements of Leung, Vass, and Gomer, which are still high by a factor of 5. The new measurements permit a recalculation of excitation cross sections for neutral desorption. It is found that the latter are substantially smaller than corresponding gas phase values.

  14. Cross sectional study of osteoporosis among women.

    PubMed

    Agrawal, Tripti; Verma, A K

    2013-04-01

    Osteoporosis is a major public health problem, associated with substantial morbidity and socio-economic burden. An early detection can help in reducing the fracture rates and overall socio-economic burden. The present study was carried out to screen the bone status (osteopenia and osteoporosis) above the age of 35 yrs in the women. A community based cross sectional study was carried out in 158 women by calculating WHO T-scores utilizing calcaneal QUS as diagnostic tool. The prevalence of osteoporosis and osteopenia was found to be 13.3% ± 5.29% and 48.1% ± 7.79% respectively. Statistical association of prevalence of osteopenia and osteoporosis was found to be significant with age group; gravida status; attainment of menopause; body weight and physically active status of the women. The statistical association was not significant in relation to the rank status of their husband, as well as dietary pattern of the women but still it has to be substantiated by conducting larger community based trials in future. The present study found that there was statistically significant relationship between age group and the prevalence of osteopenia and osteoporosis. There was a negative correlation between age of the women and BMD. Besides age, gravida status and menopausal status have negative correlation with BMD while positive correlation with physically active lifestyle. The results were found to be non-significant in relation to rank status of husband and dietary pattern.

  15. Spectroscopy and Photoabsorption Cross Sections of FNO

    NASA Astrophysics Data System (ADS)

    Burley, J. D.; Miller, C. E.; Johnston, H. S.

    1993-04-01

    The spectroscopy and photoabsorption cross sections of nitrosyl fluoride are investigated in the spectral region 350-180 nm. Results for 350-250 nm are in good agreement with the initial measurements of Johnston and Bertin and later measurements from Solgadi and Flament and Huber et al. The spectrum is assigned to a series of vibrational progressions which arise from (0, 0, 0)″ and involve excitation of the ν' 1 mode. Excitations to ( n, 0, 0)' and ( n, 0, 1)' make up the bulk of the spectrum, with promotions to ( n, 1, 0)', ( n, 0, 2)', and ( n, 1, 2)' becoming dominant at higher energies. Analysis of the spectrum results in values of ν' 1 = 1096 cm -1, ν' 2 = 480cm -1 and ν' 3 = 349 cm -1 for the excited state FNO frequencies. The experimental basis for the assignment of ν' 1 and ν' 3 is distinctly stronger than that for ν' 2. Below 250 nm, a broad, featureless continuum absorption is observed, which rises in intensity from σ = 1.77 × 10 -20cm 2 at 245 nm to 5.24 × 10 -19cm 2 at 180 nm.

  16. Abdominal sarcoidosis: cross-sectional imaging findings

    PubMed Central

    Gezer, Naciye Sinem; Başara, Işıl; Altay, Canan; Harman, Mustafa; Rocher, Laurence; Karabulut, Nevzat; Seçil, Mustafa

    2015-01-01

    Sarcoidosis is a multisystem inflammatory disease of unknown etiology. The lungs and the lymphoid system are the most commonly involved organs. Extrapulmonary involvement is reported in 30% of patients, and the abdomen is the most common extrapulmonary site with a frequency of 50%–70%. Although intra-abdominal sarcoidosis is usually asymptomatic, its presence may affect the prognosis and treatment options. The lesions are less characteristic and may mimick neoplastic or infectious diseases such as lymphoma, diffuse metastasis, and granulomatous inflammation. The liver and spleen are the most common abdominal sites of involvement. Sarcoidosis of the gastrointestinal system, pancreas, and kidneys are extremely rare. Adenopathy which is most commonly found in the porta hepatis, exudative ascites, and multiple granulomatous nodules studding the peritoneum are the reported manifestations of abdominal sarcoidosis. Since abdominal sarcoidosis is less common and long-standing, unrecognized disease can result in significant morbidity and mortality. Imaging contributes to diagnosis and management of intra-abdominal sarcoidosis. In this report we reviewed the cross-sectional imaging findings of hepatobiliary, gastrointestinal, and genitourinary sarcoidosis. PMID:25512071

  17. APPARATUS FOR MEASURING TOTAL NEUTRON CROSS SECTIONS

    DOEpatents

    Cranberg, L.

    1959-10-13

    An apparatus is described for measuring high-resolution total neutron cross sections at high counting rate in the range above 50-kev neutron energy. The pulsed-beam time-of-flight technique is used to identify the neutrons of interest which are produced in the target of an electrostatic accelerator. Energy modulation of the accelerator . makes it possible to make observations at 100 energy points simultaneously. 761O An apparatus is described for monitoring the proton resonance of a liquid which is particulariy useful in the continuous purity analysis of heavy water. A hollow shell with parallel sides defines a meander chamber positioned within a uniform magnetic fieid. The liquid passes through an inlet at the outer edge of the chamber and through a spiral channel to the central region of the chamber where an outlet tube extends into the chamber perpendicular to the magnetic field. The radiofrequency energy for the monitor is coupled to a coil positioned coaxially with the outlet tube at its entrance point within the chamber. The improvement lies in the compact mechanical arrangement of the monitor unit whereby the liquid under analysis is subjected to the same magnetic field in the storage and sensing areas, and the entire unit is shielded from external electrostatic influences.

  18. Cross-sectional imaging in Crohn disease.

    PubMed

    Furukawa, Akira; Saotome, Takao; Yamasaki, Michio; Maeda, Kiyosumi; Nitta, Norihisa; Takahashi, Masashi; Tsujikawa, Tomoyuki; Fujiyama, Yoshihide; Murata, Kiyoshi; Sakamoto, Tsutomu

    2004-01-01

    The role of cross-sectional imaging in the diagnosis of Crohn disease has expanded with recent technologic advances in computed tomography (CT) and magnetic resonance (MR) imaging that allow rapid acquisition of high-resolution images of the intestines. To acquire images of diagnostic quality, administration of a fairly large amount of intraluminal contrast agent prior to examination and scanning with intravenous contrast material injection are necessary. Both CT and MR imaging are reported to have a sensitivity of over 95% for the detection of Crohn disease; however, they may not allow early diagnosis. Colonoscopy and conventional enteroclysis studies are indicated for patients with early-stage disease. At more advanced stages, CT and MR imaging can help identify and characterize pathologically altered bowel segments as well as extraluminal lesions (eg, fistulas, abscesses, fibrofatty proliferation, increased vascularity of the vasa recta, mesenteric lymphadenopathy). These modalities can also clearly depict inflammatory lesion activity and conditions that require elective gastrointestinal surgery, thereby aiding in treatment planning. In the clinical setting, CT is currently the imaging modality of choice at most institutions; however, it is expected that MR imaging will soon play a comparable role. CT or MR imaging should be included in a comprehensive evaluation of patients with Crohn disease, along with conventional imaging and clinical and laboratory tests.

  19. [Fast neutron cross section measurements]. Progress report

    SciTech Connect

    Knoll, G.F.

    1992-10-26

    From its inception, the Nuclear Data Project at the University of Michigan has concentrated on two major objectives: (1) to carry out carefully controlled nuclear measurements of the highest possible reliability in support of the national nuclear data program, and (2) to provide an educational opportunity for students with interests in experimental nuclear science. The project has undergone a successful transition from a primary dependence on our photoneutron laboratory to one in which our current research is entirely based on a unique pulsed 14 MeV fast neutron facility. The new experimental facility is unique in its ability to provide nanosecond bursts of 14 MeV neutrons under conditions that are ``clean`` and as scatter-free as possible, and is the only one of its type currently in operation in the United States. It has been designed and put into operation primarily by graduate students, and has met or exceeded all of its important initial performance goals. We have reached the point of its routine operation, and most of the data are now in hand that will serve as the basis for the first two doctoral dissertations to be written by participating graduate students. Our initial results on double differential neutron cross sections will be presented at the May 1993 Fusion Reactor Technology Workshop. We are pleased to report that, after investing several years in equipment assembly and optimization, the project has now entered its ``data production`` phase.

  20. Nondipole effects in helium photoionization

    NASA Astrophysics Data System (ADS)

    Argenti, Luca; Moccia, Roberto

    2010-12-01

    An accurate calculation of the nondipole anisotropy parameter γ in the photoionization of helium below the N = 2 threshold is presented. The calculated results are in fairly good agreement with the experimental results of Krässig et al (2002 Phys. Rev. Lett. 88 203002), but not as good as the accuracy of the calculation should have warranted. A careful examination of the possible causes for the observed discrepancies between theory and experiment seems to rule out any role either of the multipolar terms higher than the electric quadrupole, or of the singlet-triplet spin-orbit mixing. It is argued that such discrepancies might have an instrumental origin, due to the difficulty of measuring vanishingly small total cross sections σtot with the required accuracy. In such eventuality, it might be more appropriate to use a parameter other than γ, such as for instance the drag current, to measure the nondipole anisotropy of the photoelectron angular distribution.

  1. Graphs of the cross sections in the Alternate Monte Carlo Cross Section library at the Los Alamos Scientific Laboratory

    SciTech Connect

    Seamon, R.E.; Soran, P.D.

    1980-06-01

    Graphs of all neutron cross sections and photon production cross sections on the Alternate Monte Carlo Cross Section (AMCCS) library have been plotted along with local neutron heating numbers. The values of ..nu..-bar, the average number of neutrons per fission, are also plotted for appropriate isotopes.

  2. Graphs of the cross sections in the recommended Monte Carlo cross-section library at the Los Alamos Scientific Laboratory

    SciTech Connect

    Soran, P.D.; Seamon, R.E.

    1980-05-01

    Graphs of all neutron cross sections and photon production cross sections on the Recommended Monte Carlo Cross Section (RMCCS) library have been plotted along with local neutron heating numbers. Values for anti ..nu.., the average number of neutrons per fission, are also given.

  3. Excitation cross sections for krypton by electrons in the 15-100-eV impact-energy range

    NASA Technical Reports Server (NTRS)

    Trajmar, S.; Srivastava, S. K.; Tanaka, H.; Nishimura, H.; Cartwright, D. C.

    1981-01-01

    Differential, integral, and momentum-transfer cross sections have been determined for the excitation of the 24 lowest electronic states of Kr (some of the transitions are unresolved). The inelastic-scattering cross sections were normalized to the absolute scale with the help of the elastic-scattering differential cross sections (DCS's) which in turn were normalized with respect to absolute He DCS's. The impact energies were 15, 20, 30, 50, and 100 eV and the DCS's were obtained over the range of 5-135 deg scattering angles. The error limits associated with the differential, integral, and momentum-transfer cross sections have been estimated at 25%, 38%, and 46%, respectively.

  4. The study of state-selected ion-molecule reactions using the vacuum ultraviolet pulsed field ionization-photoion technique.

    PubMed

    Dressler, Rainer A; Chiu, Y; Levandier, D J; Tang, X N; Hou, Y; Chang, C; Houchins, C; Xu, H; Ng, Cheuk-Yiu

    2006-10-07

    This paper presents the methodology to generate beams of ions in single quantum states for bimolecular ion-molecule reaction dynamics studies using pulsed field ionization (PFI) of atoms or molecules in high-n Rydberg states produced by vacuum ultraviolet (VUV) synchrotron or laser photoexcitation. Employing the pseudocontinuum high-resolution VUV synchrotron radiation at the Advanced Light Source as the photoionization source, PFI photoions (PFI-PIs) in selected rovibrational states have been generated for ion-molecule reaction studies using a fast-ion gate to pass the PFI-PIs at a fixed delay with respect to the detection of the PFI photoelectrons (PFI-PEs). The fast ion gate provided by a novel interleaved comb wire gate lens is the key for achieving the optimal signal-to-noise ratio in state-selected ion-molecule collision studies using the VUV synchrotron based PFI-PE secondary ion coincidence (PFI-PESICO) method. The most recent development of the VUV laser PFI-PI scheme for state-selected ion-molecule collision studies is also described. Absolute integral cross sections for state-selected H2+ ions ranging from v+ = 0 to 17 in collisions with Ar, Ne, and He at controlled translational energies have been obtained by employing the VUV synchrotron based PFI-PESICO scheme. The comparison between PFI-PESICO cross sections for the H2+(HD+)+Ne and H2+(HD+)+He proton-transfer reactions and theoretical cross sections based on quasiclassical trajectory (QCT) calculations and three-dimensional quantum scattering calculations performed on the most recently available ab initio potential energy surfaces is highlighted. In both reaction systems, quantum scattering resonances enhance the integral cross sections significantly above QCT predictions at low translational and vibrational energies. At higher energies, the agreement between experiment and quasiclassical theory is very good. The profile and magnitude of the kinetic energy dependence of the absolute integral cross

  5. Vibrational-excitation cross sections of water molecules by electron impact

    NASA Technical Reports Server (NTRS)

    Shyn, T. W.; Cho, S. Y.; Cravens, T. E.

    1988-01-01

    A crossed-beam technique was used to measure absolute differential cross sections for the vibrational excitation of water-vapor molecules. The energy and angular range were from 2.2 to 20 eV and from 30 to 150 deg. Vibrational-excitation cross sections were determined for the bending (010) and stretching (100 and 001) modes of the electronic ground state. It is shown that the integral cross sections are generally larger than those of Seng and Linder (1976) by 10-20 percent for both the bending and stretching modes. It is noted that the results obtained are of interest in connection with the theoretical modeling of cometary ionospheres.

  6. Cross sections for elastic electron scattering by tetramethylsilane in the intermediate-energy range

    SciTech Connect

    Sugohara, R. T.; Lee, M.-T.; Iga, I.; Souza, G. L. C. de; Homem, M. G. P.

    2011-12-15

    Organosilicon compounds are of current interest due to the numerous applications of these species in industries. Some of these applications require the knowledge of electron collision cross sections, which are scarce for such compounds. In this work, we report absolute values of differential, integral, and momentum-transfer cross sections for elastic electron scattering by tetramethylsilane (TMS) measured in the 100-1000 eV energy range. The relative-flow technique is used to normalize our data. In addition, the independent-atom-model (IAM) and the additivity rule (AR), widely used to model electron collisions with light hydrocarbons, are also applied for e{sup -}-TMS interaction. The comparison of our measured results of cross sections and the calculated data shows good agreement, particularly near the higher-end of incident energies.

  7. First Measurement of the Muon Neutrino Charged Current Quasielastic Double Differential Cross Section

    SciTech Connect

    Aguilar-Arevalo, A.A.; Anderson, C.E.; Bazarko, A.O.; Brice, S.J.; Brown, B.C.; Bugel, L.; Cao, J.; Coney, L.; Conrad, J.M.; Cox, D.C.; Curioni, A.; /Yale U. /Columbia U.

    2010-02-01

    A high-statistics sample of charged-current muon neutrino scattering events collected with the MiniBooNE experiment is analyzed to extract the first measurement of the double differential cross section (d{sup 2}{sigma}/dT{sub {mu}}d cos {theta}{sub {mu}}) for charged-current quasielastic (CCQE) scattering on carbon. This result features minimal model dependence and provides the most complete information on this process to date. With the assumption of CCQE scattering, the absolute cross section as a function of neutrino energy ({sigma}[E{sub {nu}}]) and the single differential cross section (d{sigma}/dQ{sup 2}) are extracted to facilitate comparison with previous measurements. These quantities may be used to characterize an effective axial-vector form factor of the nucleon and to improve the modeling of low-energy neutrino interactions on nuclear targets. The results are relevant for experiments searching for neutrino oscillations.

  8. Electron-impact ionization cross sections out of the ground and excited states of cesium

    SciTech Connect

    Lukomski, M.; Sutton, S.; Kedzierski, W.; Reddish, T. J.; Bartschat, K.; Bartlett, P. L.; Bray, I.; Stelbovics, A. T.; McConkey, J. W.

    2006-09-15

    An atom trapping technique for determining absolute, total ionization cross sections (TICS) out of an excited atom is presented. The unique feature of our method is in utilizing Doppler cooling of neutral atoms to determine ionization cross sections. This fluorescence-monitoring experiment, which is a variant of the 'trap loss' technique, has enabled us to obtain the experimental electron impact ionization cross sections out of the Cs state between 7 eV and 400 eV. CCC, RMPS, and Born theoretical results are also presented for both the ground and excited states of cesium and rubidium. In the low energy region (<11 eV) where best agreement between these excited state measurements and theory might be expected, a discrepancy of approximately a factor of five is observed. Above this energy there are significant contributions to the TICS from both autoionization and multiple ionization.

  9. Measurement of the Proton + Proton Going to Proton + Proton + Neutral Pion Cross-Section Near Threshold

    NASA Astrophysics Data System (ADS)

    Ross, M. Alan

    1991-02-01

    The first nuclear physics experiment at the IUCF Cooler is a measurement of the p+ptop+p+ pi^0 cross section near threshold. The Cooler, together with a thin internal H_2 gas jet target, allows for a precise cross section measurement by providing well-defined interaction energies and by eliminating background from p-nucleus pion production which has a much lower threshold. A cylindrically symmetric detector system has been installed in one of the straight sections of the ring and is used to detect the coincident protons in the exit channel with good energy and angular resolution. The mass of the unobserved is then deduced. Elastically scattered protons were detected at the same time and by the same detector as pion production events. Elastic scattering was used for normalization to obtain an absolute p+p top+p+pi^0 cross section.

  10. Probing insect backscatter cross-section and melanization using kHz optical remote detection system

    NASA Astrophysics Data System (ADS)

    Gebru, Alem K.; Brydegaard, Mikkel; Rohwer, Erich; Neethling, Pieter

    2016-09-01

    kHz optical remote sensing system is implemented to determine melanization and backscatter cross-section in the near infrared (NIR) and shortwave infrared (SWIR) in situ. It is shown that backscatter cross-section in the SWIR is insensitive to melanization and absolute melanization can be derived from the ratio of backscatter cross-section in two bands (SWIR/NIR). We have shown that insects reflect more strongly in the SWIR as compared to NIR and Visible (VIS) in accordance with previous findings. This is illustrated using three different insects (Snow white moth (spilosoma genus), Fox moth (Macrothylacia) and Leather beetle (Odontotaenius genus)) and it is shown that the reflectance of the Leather beetle in the VIS and NIR is more affected by melanization as compared with snow white moth.

  11. State selective photo-recombination cross sections in Be-like C and Al ions

    NASA Astrophysics Data System (ADS)

    Stancalie, Viorica

    2013-11-01

    We report results from detailed state selective photo-recombination study along with the doubly excited autoionizing resonances in Be-like C2+ and Al9+ ions. In the present investigation, the primary focus is on detailed energy profiles of the individual photo-recombination cross sections. The calculation was carried out for the excited Rydberg states of type 1 s 22 sns(1Se) which interact with the odd-parity continua up to the C3+ and Al10+ 2 p threshold limit. The numerical evaluation has been performed at a fine energy mesh across all the autoionizing Rydberg series of resonances 1 s 22 pns(1P0) converging to Li-like ion 2 p threshold. The method of calculation keeps the essential ingredients of the Feshbach projection operator approximation. The photo-ionization cross sections have been evaluated with and without relativistic effects included into the R-matrix numerical procedures, while the allowance for both quantum interference between dielectronic and radiative recombination, and overlapping resonances has been done utilizing results from the earlier R-matrix Floquet calculation. We discuss all these results with respect to the effect of quantum interference term on the energy dependence profile of photo-recombination cross section for studied transitions.

  12. Studies of the dependence of the microwave radar cross section on ocean surface variables during the FASINEX experiment

    NASA Technical Reports Server (NTRS)

    Weissman, D. A.; Li, Fuk

    1988-01-01

    The ability of theoretical radar cross section (RCS) models to predict the absolute magnitude of the ocean radar cross section under a wide variety of sea and atmospheric conditions was studied using experimental data from the FASINEX Experiment. This consists of RCS data from a Ku-band scatterometer mounted on an aircraft (10 separate flights were conducted), a wide variety of atmospheric measurements (including stress) and sea conditions. Theoretical models are tested. Where discrepancies are observed, revisions are hypothesized and evaluated.

  13. Measurement of the nu(mu)-CCQE cross-section in the SciBooNE experiment

    SciTech Connect

    Alcaraz-Aunion, Jose Luis; Walding, Joseph; /Imperial Coll., London

    2009-09-01

    SciBooNE is a neutrino and anti-neutrino cross-section experiment at Fermilab, USA. The SciBooNE experiment is summarized and two independent CCQE analyses are described. For one of the analyses, an absolute {nu}{sub {mu}}-CCQE cross section in the neutrino energy region (0.6-1.6) GeV is shown and the technique developed for such a purpose is also explained. The total cross section measured over this energy range agrees well with expectations, based on the NEUT event generator and using a value of 1.21 GeV for the CCQE axial mass.

  14. Allergic conjunctivitis: a cross-sectional study.

    PubMed

    Leonardi, A; Piliego, F; Castegnaro, A; Lazzarini, D; La Gloria Valerio, A; Mattana, P; Fregona, I

    2015-06-01

    Ocular allergy is a common disease in daily practice. A cross-sectional study was conducted to evaluate clinical aspects of and therapeutic approaches to ocular allergy in Italy. Of the 3685 patients affected by ocular allergy and enrolled by 304 ophthalmologists nationally, 3545 were eligible to be included in the statistical analysis. A questionnaire was administered in office to record demographic data, comorbidities, trigger factors, number of conjunctivitis episodes, and past treatments. Signs and symptoms were graded according to their severity, frequency, and duration. Mean age of enrolled patients was 38 ± 19 years. Seasonal allergic conjunctivitis (55% of patients) was equally distributed among the different age groups, while perennial allergic conjunctivitis (18%) increased with age and vernal keratoconjunctivitis (9%) was more frequent under the age of 18. Itching and redness were reported in 90% and 85%, respectively; lid skin involvement was observed in 22% of cases and keratitis in 11%. Pollen sensitivities were indicated as the most frequent triggers; however, exposure to non-specific environmental conditions, pollutants, and cigarette smoke was frequently reported. Only 35% of patients underwent a diagnostic evaluation of specific allergic sensitization, with positive allergy tests found in 82% of this subset. With regard to treatment, topical decongestants were used in 43% of patients, corticosteroids in 41%, antihistamines in 29%, systemic antihistamines in 27%, and mast cell stabilizers in 15%. This survey provided useful epidemiological information regarding the clinical characteristics and treatment options of a large cohort of patients affected by different forms of ocular allergy. An understanding of ocular allergic disease, its incidence, demographics, and treatment paradigms provides important information towards understanding its pharmacoeconomics and burden on the national health system. © 2015 John Wiley & Sons Ltd.

  15. Photoionization of chlorine-like potassium and calcium ions

    NASA Astrophysics Data System (ADS)

    Alna'Washi, Ghassan A.

    Absolute photoionization cross-section measurements were performed for a mixture of 2Po 3/2 ground state and 2Po 1/2 metastable state Cl-like K2+ and Ca3+ ions over the photon energy range 44.240-69.741 eV for K2+ and 65.7-104.6 eV for Ca3+. The measurements were performed by merging an ion beam with a beam of synchrotron radiation from an undulator magnet using the ion-photon merged-beams endstation on beamline 10.0.1 of the Advanced Light Source (ALS) at Lawrence Berkley National Laboratory. High resolution measurements were performed near the 2P o 3/2 ground-state ionization threshold for both ions. The ground-state ionization thresholds of K2+ and Ca 3+ was measured to be 45.740 +/- 0.015 eV and 67.070 +/- 0.018 eV, respectively. These energies are respectively 0.066 eV and 0.200 eV lower than the tabulated values in the NIST database. These data are compared to previous measurements for Cl-like Ar+. Most of the observed resonance features belong to multiple Rydberg series of transitions to autoionizing states. These features were assigned spectroscopically using the quantum defect form of the Rydberg formula, guided by calculations of the energies and oscillator strengths of transitions to autoionizing states performed using the pseudo-relativistic Cowan Hartree-Fock atomic structure code. The measurements for Ca3+ compare favorably with recent unpublished R-matrix calculations performed by McLaughlin in a close-coupling expansion within the semi-relativistic Breit-Pauli approximation. This includes the energy positions of the calculated resonances and the magnitudes of the resonant and nonresonant components of the cross section.

  16. A probabilistic methodology for radar cross section prediction in conceptual aircraft design

    NASA Astrophysics Data System (ADS)

    Hines, Nathan Robert

    System effectiveness has increasingly become the prime metric for the evaluation of military aircraft. As such, it is the decision maker's/designer's goal to maximize system effectiveness. Industry and government research documents indicate that all future military aircraft will incorporate signature reduction as an attempt to improve system effectiveness and reduce the cost of attrition. Today's operating environments demand low observable aircraft which are able to reliably take out valuable, time critical targets. Thus it is desirable to be able to design vehicles that are balanced for increased effectiveness. Previous studies have shown that shaping of the vehicle is one of the most important contributors to radar cross section, a measure of radar signature, and must be considered from the very beginning of the design process. Radar cross section estimation should be incorporated into conceptual design to develop more capable systems. This research strives to meet these needs by developing a conceptual design tool that predicts radar cross section for parametric geometries. This tool predicts the absolute radar cross section of the vehicle as well as the impact of geometry changes, allowing for the simultaneous tradeoff of the aerodynamic, performance, and cost characteristics of the vehicle with the radar cross section. Furthermore, this tool can be linked to a campaign theater analysis code to demonstrate the changes in system and system of system effectiveness due to changes in aircraft geometry. A general methodology was developed and implemented and sample computer codes applied to prototype the proposed process. Studies utilizing this radar cross section tool were subsequently performed to demonstrate the capabilities of this method and show the impact that various inputs have on the outputs of these models. The F/A-18 aircraft configuration was chosen as a case study vehicle to perform a design space exercise and to investigate the relative impact of

  17. IONIS: Approximate atomic photoionization intensities

    NASA Astrophysics Data System (ADS)

    Heinäsmäki, Sami

    2012-02-01

    A program to compute relative atomic photoionization cross sections is presented. The code applies the output of the multiconfiguration Dirac-Fock method for atoms in the single active electron scheme, by computing the overlap of the bound electron states in the initial and final states. The contribution from the single-particle ionization matrix elements is assumed to be the same for each final state. This method gives rather accurate relative ionization probabilities provided the single-electron ionization matrix elements do not depend strongly on energy in the region considered. The method is especially suited for open shell atoms where electronic correlation in the ionic states is large. Program summaryProgram title: IONIS Catalogue identifier: AEKK_v1_0 Program summary URL:http://cpc.cs.qub.ac.uk/summaries/AEKK_v1_0.html Program obtainable from: CPC Program Library, Queen's University, Belfast, N. Ireland Licensing provisions: Standard CPC licence, http://cpc.cs.qub.ac.uk/licence/licence.html No. of lines in distributed program, including test data, etc.: 1149 No. of bytes in distributed program, including test data, etc.: 12 877 Distribution format: tar.gz Programming language: Fortran 95 Computer: Workstations Operating system: GNU/Linux, Unix Classification: 2.2, 2.5 Nature of problem: Photoionization intensities for atoms. Solution method: The code applies the output of the multiconfiguration Dirac-Fock codes Grasp92 [1] or Grasp2K [2], to compute approximate photoionization intensities. The intensity is computed within the one-electron transition approximation and by assuming that the sum of the single-particle ionization probabilities is the same for all final ionic states. Restrictions: The program gives nonzero intensities for those transitions where only one electron is removed from the initial configuration(s). Shake-type many-electron transitions are not computed. The ionized shell must be closed in the initial state. Running time: Few seconds for a

  18. Integral elastic, electronic-state, ionization, and total cross sections for electron scattering with furfural

    NASA Astrophysics Data System (ADS)

    Jones, D. B.; da Costa, R. F.; Varella, M. T. do N.; Bettega, M. H. F.; Lima, M. A. P.; Blanco, F.; García, G.; Brunger, M. J.

    2016-04-01

    We report absolute experimental integral cross sections (ICSs) for electron impact excitation of bands of electronic-states in furfural, for incident electron energies in the range 20-250 eV. Wherever possible, those results are compared to corresponding excitation cross sections in the structurally similar species furan, as previously reported by da Costa et al. [Phys. Rev. A 85, 062706 (2012)] and Regeta and Allan [Phys. Rev. A 91, 012707 (2015)]. Generally, very good agreement is found. In addition, ICSs calculated with our independent atom model (IAM) with screening corrected additivity rule (SCAR) formalism, extended to account for interference (I) terms that arise due to the multi-centre nature of the scattering problem, are also reported. The sum of those ICSs gives the IAM-SCAR+I total cross section for electron-furfural scattering. Where possible, those calculated IAM-SCAR+I ICS results are compared against corresponding results from the present measurements with an acceptable level of accord being obtained. Similarly, but only for the band I and band II excited electronic states, we also present results from our Schwinger multichannel method with pseudopotentials calculations. Those results are found to be in good qualitative accord with the present experimental ICSs. Finally, with a view to assembling a complete cross section data base for furfural, some binary-encounter-Bethe-level total ionization cross sections for this collision system are presented.

  19. Cross sections for inelastic collisions of fast charged particles with atoms and molecules

    SciTech Connect

    Inokuti, Mitio

    1985-01-01

    A large volume of data of these cross sections are required for solving problems of radiological physics and dosimetry, as well as for detailed analysis of the earliest stage of radiation actions on matter (including the biological cell and substances constituting it). Current experimental data of the cross sections are far from being complete or even satisfactory for tentative applications. One practical approach to the cross-section determination is to test experimental data with general criteria. For example, the Bethe theory indicates a close connection between photoabsorption and energy absorption by glancing collisions. Development and use of these data constraints, first put forth by Platzman, can now be demonstrated in many examples. More recent studies concern the determination of the analytic expression most suitable for fitting the data on the oscillator-strength distribution or the energy distribution of secondary electrons from ionizing collisions of charged particles. There are three areas to which major efforts should be directed. First, methods of absolute cross-section measurements both for electron and ionic collisions must be thoroughly reviewed so that sources of systematic errors may be identified and corrected. Second, efforts should be devoted to the understanding of the data systematics, viz., the trends of cross sections for a series of molecules. Finally, electron and ionic collisions with molecules in condensed phases will be an important topic of study for years to come; initial reports on efforts toward this direction are encouraging. 46 refs.

  20. Positron-impact ionization, positronium formation, and electronic excitation cross sections for diatomic molecules

    SciTech Connect

    Marler, J. P.; Surko, C. M.

    2005-12-15

    Absolute measurements are presented for the positron-impact cross sections for positronium formation, direct ionization, and total ionization of the diatomic molecules N{sub 2}, CO, and O{sub 2}, in the range of energies from threshold to 90 eV. Cross sections for the electronic excitation of the a {sup 1}{pi} and a{sup '} {sup 1}{sigma} state in N{sub 2} and the A {sup 1}{pi} state in CO near threshold are also presented. The experiment uses a cold, trap-based positron beam and the technique of studying positron scattering in a strong magnetic field. In O{sub 2}, a feature previously seen in the total ionization cross section is observed in both the positronium formation and total ionization cross sections. The possible origin of this feature and its relationship to positron-induced dissociation is discussed. In N{sub 2}, the near-threshold electronic excitation cross section is larger than that for positronium formation. This likely explains the relatively high efficiency of this molecule when used for buffer-gas positron trapping.

  1. Forward pd elastic scattering and total spin-dependent pd cross sections at intermediate energies

    SciTech Connect

    Uzikov, Yu. N.; Haidenbauer, J.

    2009-02-15

    Spin-dependent total pd cross sections are considered using the optical theorem. For this aim the full spin dependence of the forward pd elastic scattering amplitude is considered in a model independent way. The single-scattering approximation is used to relate this amplitude to the elementary amplitudes of pp and pn scattering and the deuteron form factor. A formalism allowing to take into account Coulomb-nuclear interference effects in polarized pd cross sections is developed. Numerical calculations for the polarized total pd cross sections are performed at beam energies 20-300 MeV using the NN interaction models developed by the Juelich group. Double-scattering effects are estimated within the Glauber approach and found to be in the order of 10-20%. Existing experimental data on differential pd cross sections are in good agreement with the performed Glauber calculations. It is found that for the used NN models the total longitudinal and transversal pd cross sections are comparable in absolute value to those for pp scattering.

  2. Influence of screening length modification on the scattering cross section in LEIS

    NASA Astrophysics Data System (ADS)

    Primetzhofer, D.; Markin, S. N.; Efrosinin, D. V.; Steinbauer, E.; Andrzejewski, R.; Bauer, P.

    2011-06-01

    Scattering cross sections for He + ions in the energy range of 100 eV to 100 keV and for Al, Cu and Au target atoms were calculated. Employing the Thomas-Fermi-Molière model the potential strength was tuned by variation of the screening length. The resulting change in scattering cross section was analyzed and the absolute value is compared to cross sections obtained from potentials commonly employed in the medium-energy ion scattering (MEIS) regime. A large influence on the scattering cross section is observed for targets with large atomic number in the very low energy range. For instance, the scattering cross section for 100 eV He +-ions scattered from Au by 129° changes by a factor of 2.5 between different potential strengths claimed in the literature to be suitable for low-energy ion scattering (LEIS) energies. An experiment to determine electronic energy loss of very slow ions in metals is presented. It shows how uncertainties in the scattering potential strength can lead to systematically wrong results, although perfect agreement between experimental data and simulations is found. The impact of these results on quantitative surface structure and composition analysis is discussed.

  3. Photoionization of hydrogen-like ions in dense quantum plasmas

    NASA Astrophysics Data System (ADS)

    Qi, Y. Y.; Wang, J. G.; Janev, R. K.

    2017-06-01

    The photoionization of hydrogen-like ions in n ≤ 3 bound states, embedded in cold, dense quantum plasmas, is investigated in detail. The electron energies and wave functions for the bound and continuum states are determined by numerically solving the scaled Schrödinger equation by the fourth-order symplectic integration scheme. The monotonic behavior of the photoionization cross section for a pure Coulomb potential is dramatically changed due to the plasma screening effects described by the cosine-Debye-Hückel potential. In the region of low photoelectron energies, the photoionization cross section, besides the usual Wigner-law threshold behavior, exhibits a rich structure of shape and virtual-state resonances when the plasma screening parameter takes values around the critical screening parameter for which a bound state enters the continuum. It is observed that a shape resonance is followed by a Cooper minimum in the photoionization cross section when the principal quantum number of continuum quasi-bound state is equal to the one of the initial bound states.

  4. Crosstalk in rectangular cross-section heterogeneous multicore fiber

    NASA Astrophysics Data System (ADS)

    Egorova, Olga N.; Astapovich, Maxim S.; Semjonov, Sergey L.

    2016-09-01

    Using neighboring cores with different mode propagation constants (indexes) is a well-known way to reduce crosstalk in multicore fiber (MCF). However, in actual field-deployed fiber, random bends can cause a reduction in the difference between the mode indexes of neighboring cores, which consequently increases crosstalk. The level of crosstalk induced by bending in both rectangular cross-section and circular cross-section heterogeneous MCF with cores arranged in a line was investigated. The experimental results obtained indicate that in contrast to circular cross-section MCF, no bending-induced crosstalk occurs in rectangular cross-section MCF wound on the mandrel without special control of cross-section orientation. Thus, to eliminate undesirable bending-induced crosstalk in heterogeneous MCF a rectangular cross-section should be employed.

  5. Partial Photoneutron Cross Sections for 207,208Pb

    NASA Astrophysics Data System (ADS)

    Kondo, T.; Utsunomiya, H.; Goriely, S.; Iwamoto, C.; Akimune, H.; Yamagata, T.; Toyokawa, H.; Harada, H.; Kitatani, F.; Lui, Y.-W.; Hilaire, S.; Koning, A. J.

    2014-05-01

    Using linearly-polarized laser-Compton scattering γ-rays, partial E1 and M1 photoneutron cross sections along with total cross sections were determined for 207,208Pb at four energies near neutron threshold by measuring anisotropies in photoneutron emission. Separately, total photoneutron cross sections were measured for 207,208Pb with a high-efficiency 4π neutron detector. The partial cross section measurement provides direct evidence for the presence of pygmy dipole resonance (PDR) in 207,208Pb in the vicinity of neutron threshold. The strength of PDR amounts to 0.32%-0.42% of the Thomas-Reiche-Kuhn sum rule. Several μN2 units of B(M1)↑ strength were observed in 207,208Pb just above neutron threshold, which correspond to M1 cross sections less than 10% of the total photoneutron cross sections.

  6. Color dipole cross section and inelastic structure function

    NASA Astrophysics Data System (ADS)

    Jeong, Yu Seon; Kim, C. S.; Luu, Minh Vu; Reno, Mary Hall

    2014-11-01

    Instead of starting from a theoretically motivated form of the color dipole cross section in the dipole picture of deep inelastic scattering, we start with a parametrization of the deep inelastic structure function for electromagnetic scattering with protons, and then extract the color dipole cross section. Using the parametrizations of F 2(ξ = x or W 2 , Q 2) by Donnachie-Landshoff and Block et al., we find the dipole cross section from an approximate form of the presumed dipole cross section convoluted with the perturbative photon wave function for virtual photon splitting into a color dipole with massless quarks. The color dipole cross section determined this way reproduces the original structure function within about 10% for 0 .1 GeV2 ≤ Q 2 ≤10 GeV2. We discuss the dipole cross section at large and small dipole sizes and compare our results with other parametrizations.

  7. Total and partial photoneutron cross sections for Pb isotopes

    NASA Astrophysics Data System (ADS)

    Kondo, T.; Utsunomiya, H.; Goriely, S.; Daoutidis, I.; Iwamoto, C.; Akimune, H.; Okamoto, A.; Yamagata, T.; Kamata, M.; Itoh, O.; Toyokawa, H.; Lui, Y.-W.; Harada, H.; Kitatani, F.; Hilaire, S.; Koning, A. J.

    2012-07-01

    Using quasimonochromatic laser-Compton scattering γ rays, total photoneutron cross sections were measured for 206,207,208Pb near neutron threshold with a high-efficiency 4π neutron detector. Partial E1 and M1 photoneutron cross sections along with total cross sections were determined for 207,208Pb at four energies near threshold by measuring anisotropies in photoneutron emission with linearly polarized γ rays. The E1 strength dominates over the M1 strength in the neutron channel where E1 photoneutron cross sections show extra strength of the pygmy dipole resonance in 207,208Pb near the neutron threshold corresponding to 0.32%-0.42% of the Thomas-Reiche-Kuhn sum rule. Several μN2 units of B(M1)↑ strength were observed in 207,208Pb just above neutron threshold, which correspond to an M1 cross section less than 10% of the total photoneutron cross section.

  8. Coupled multigroup cross sections for hydrogen interactions in plasmas

    NASA Astrophysics Data System (ADS)

    Wienke, B. R.; Morel, J. E.; Cayton, T. E.; Howell, R. B.

    1985-10-01

    Using analytical fits to the experimental cross sections for H 3 H 2, and H 2+ interactions in plasmas, developed by Gryzinski, Riviere, Jones, and Freeman, we obtain coupled multigroup cross sections and rate coefficients for hydrogen transport applications. Multigroup cross sections and rate coefficients, for specified energy group boundaries, plasma particle and temperature profiles, and cylindrical plasma confinement radius, are generated against a spatially dependent, local Maxwellian scattering background. Cross sections are formatted for direct use in production multigroup S n, Monte Carlo, or specific transport applications. Ten coupled hydrogen reactions are included and resulting cross sections for ionization, scattering, and production can be coupled or decoupled. Reactions treated include H, H 2 ionization by electrons and protons, H, H 2 charge exchange, and H 2, H 2+ dissociative mechanisms. We detail the formalism used to compute effective cross sections and rates and give practicle results for two fusion reactors.

  9. Theoretical Fully Differential Cross Sections for Four-Body Processes

    NASA Astrophysics Data System (ADS)

    Harris, A. L.; Peacher, J. L.; Schulz, M.; Madison, D. H.

    2008-04-01

    Atomic collisions present a valuable opportunity to study the few body problem. Advances on the theoretical side now allow for an essentially exact numerical calculation of one of the simplest the few-body problems - the three-body problem. However, study of the four-body problem is still in its infancy, and the agreement between experiment and theory for kinematically complete experiments is far from satisfactory. The simplest four-body problem is a charged particle collision with helium in which both atomic electrons change state. Two theoretical models will be discussed for several possible outcomes of this type of collision. The first Born approximation (FBA) treats the projectile as a plane wave, and ignores the post collision Coulomb interaction between the two final state continuum electrons. The more sophisticated four-body distorted wave (4DW) model treats all continuum particles as distorted waves and explicitly includes the post collision Coulomb interaction between the two outgoing electrons. Fully differential cross sections calculated using the FBA and 4DW models will be compared to absolute experimental results, as well as other theories.

  10. Awareness of surgical costs: a multicenter cross-sectional survey.

    PubMed

    Bade, Kim; Hoogerbrug, Jonathan

    2015-01-01

    Resource scarcity continues to be an important problem in modern surgical practice. Studies in North America and Europe have found that medical professionals have limited understanding of the costs of medical care. No cost awareness studies have been undertaken in Australasia or specifically focusing on the surgical team. This study determined the cost of a range of commonly used diagnostic tests, procedures, and hospital resources associated with care of the surgical patient. The surgical teams' awareness of these costs was then assessed in a multicenter cross-sectional survey. In total, 14 general surgical consultants, 14 registrars, and 25 house officers working in three New Zealand hospitals were asked to estimate the costs of 14 items commonly associated with patient care. Cost estimations were considered correct if within 25% plus or minus of the actual cost. Accuracy was assessed by calculating the median, mean, and absolute percentage discrepancy. A total of 57 surveys were completed. Of which, four were incomplete and were not included in the analysis. Cost awareness was generally poor, and members of the surgical team were rarely able to estimate the costs to within 25%. The mean absolute percentage error was 0.87 (95% CI: 0.58-1.18) and underestimates were most common. There was no significant difference in estimate accuracy between consultants, registrars, or house officers, or between consultants working in both public/private practice compared with those working in public practice alone. There is poor awareness of surgical costs among consultant surgeons, registrars, and junior physicians working in Australasia. Copyright © 2014 Association of Program Directors in Surgery. Published by Elsevier Inc. All rights reserved.

  11. Photoionization of atomic hydrogen in electric field

    SciTech Connect

    Gorlov, Timofey V; Danilov, Viatcheslav V

    2010-01-01

    Laser assisted ionization of high energy hydrogen beams in magnetic fields opens wide application possibilities in accelerator physics and other fields. The key theoretical problem of the method is the calculation of the ionization probability of a hydrogen atom affected by laser and static electric fields in the particle rest frame. A method of solving this problem with the temporal Schr dinger equation including a continuum spectrum is presented in this paper in accurate form for the first time. This method allows finding the temporal evolution of the wave function of the hydrogen atom as a function of laser and static electric fields. Solving the problem of photoionization reveals quantum effects that cannot be described by the cross sectional approach. The effects play a key role in the problems of photoionization of H0 beams with the large angular or energy spread.

  12. Projectile and Lab Frame Differential Cross Sections for Electromagnetic Dissociation

    NASA Technical Reports Server (NTRS)

    Norbury, John W.; Adamczyk, Anne; Dick, Frank

    2008-01-01

    Differential cross sections for electromagnetic dissociation in nuclear collisions are calculated for the first time. In order to be useful for three - dimensional transport codes, these cross sections have been calculated in both the projectile and lab frames. The formulas for these cross sections are such that they can be immediately used in space radiation transport codes. Only a limited amount of data exists, but the comparison between theory and experiment is good.

  13. Left atrial vascularised thrombus diagnosed by transoesophageal cross sectional echocardiography.

    PubMed Central

    Taams, M A; Gussenhoven, E J; Lancée, C T

    1987-01-01

    This report describes a patient with a Björk-Shiley mitral valve prosthesis in whom transoesophageal cross sectional echocardiography revealed a large vascularised mass within the left atrial appendage with smoke-like opacification of blood flow in the left atrium. Transoesophageal cross sectional echocardiography gave a detailed image of the lesion which was unobtainable with precordial cross sectional echocardiography. Images Fig 1 Fig 2 PMID:3426904

  14. Measured microwave scattering cross sections of three meteorite specimens

    NASA Technical Reports Server (NTRS)

    Hughes, W. E.

    1972-01-01

    Three meteorite specimens were used in a microwave scattering experiment to determine the scattering cross sections of stony meteorites and iron meteorites in the frequency range from 10 to 14 GHz. The results indicate that the stony meteorites have a microwave scattering cross section that is 30 to 50 percent of their projected optical cross section. Measurements of the iron meteorite scattering were inconclusive because of specimen surface irregularities.

  15. Analytical formulation of the quantum electromagnetic cross section

    NASA Astrophysics Data System (ADS)

    Brandsema, Matthew J.; Narayanan, Ram M.; Lanzagorta, Marco

    2016-05-01

    It has been found that the quantum radar cross section (QRCS) equation can be written in terms of the Fourier transform of the surface atom distribution of the object. This paper uses this form to provide an analytical formulation of the quantum radar cross section by deriving closed form expressions for various geometries. These expressions are compared to the classical radar cross section (RCS) expressions and the quantum advantages are discerned from the differences in the equations. Multiphoton illumination is also briefly discussed.

  16. High E{sub T} jet cross sections at CDF

    SciTech Connect

    Flaugher, B.; CDF Collaboration

    1996-08-01

    The inclusive jet cross section for {ital p}{ital {anti p}} collisions at {radical}s = 1.8 TeV as measured by the CDF collaboration will be presented. Preliminary CDF measurements of the {Sigma} E{sub T} cross section at {radical}s = 1.8 TeV and the central inclusive jet cross section at {radical}s = 0.630 TeV will also be shown.

  17. Cross section dependence of event rates at neutrino telescopes.

    PubMed

    Hussain, S; Marfatia, D; McKay, D W; Seckel, D

    2006-10-20

    We examine the dependence of event rates at neutrino telescopes on the neutrino-nucleon cross section for neutrinos with energy above 1 PeV, and contrast the results with those for cosmic ray experiments. Scaling of the standard model cross sections leaves the rate of upward events essentially unchanged. Details, such as detector depth and cross section inelasticity, can influence rates. Numerical estimates of upward shower, muon, and tau event rates in the IceCube detector confirm these results.

  18. Giant dipole resonance parameters with uncertainties from photonuclear cross sections

    NASA Astrophysics Data System (ADS)

    Plujko, V. A.; Capote, R.; Gorbachenko, O. M.

    2011-09-01

    Updated values and corresponding uncertainties of isovector giant dipole resonance (IVGDR or GDR) model parameters are presented that are obtained by the least-squares fitting of theoretical photoabsorption cross sections to experimental data. The theoretical photoabsorption cross section is taken as a sum of the components corresponding to excitation of the GDR and quasideuteron contribution to the experimental photoabsorption cross section. The present compilation covers experimental data as of January 2010.

  19. Capture cross sections from (p,d) reactions

    NASA Astrophysics Data System (ADS)

    Escher, J. E.; Burke, J. T.; Casperson, R. J.; Hughes, R. O.; Ota, S.; Scielzo, N. D.

    2017-09-01

    Cross sections for compound-nuclear reactions involving unstable targets are important for many applications, but can often not be measured directly. Several indirect methods have been proposed to determine neutron capture cross sections for unstable isotopes. We consider an approach that aims at constraining statistical calculations of capture cross sections with data obtained from light-ion transfer reactions such as (p,d). We discuss the theoretical descriptions that have to be developed in order to extract meaningful cross section constraints from such data and show some benchmark results.

  20. Flow in tubes of non-circular cross-sections

    NASA Astrophysics Data System (ADS)

    Quadir, Raushan Ara

    Laminar, viscous, incompressible flow in tubes of noncircular cross sections is investigated. The specific aims of the investigation are (1) to look at the problems of both developing flow and fully developed flow, (2) to consider noncircular cross sections in a more systematic manner than has been done in the past, and (3) to develop a relatively simple finite element technique for producing accurate numerical solutions of flow in tubes of fairly arbitrary cross sections. Fully developed flow in tubes is governed by a Poisson type equation for the mainstream velocity. Both analytical and numerical solutions are considered. The cross sections studied include elliptic and rectangular cross sections of different aspect ratios, some triangular cross sections, and a series of crescent-shaped cross sections. The physical characteristics of the flow are examined in a systematic manner in order to determine how these characteristics are affected by certain geometrical features of the cross section. Solutions fall into three basic categories depending on the shape of the cross section. In the first category, which includes circular and elliptic cross sections, solutions are possible in closed form. In the second, including rectangular and some triangular cross sections, solutions are in the form of infinite series. In the third, including cross sections of more complicated or irregular shapes, only numerical solutions are possible. Results of calculations of velocity profiles, flow rate, pumping power, and friction factor are presented in a way which can be useful for engineering applications. In numerical studies of both developing and fully developed flow finite element techniques are used. Results are obtained for tubes of rectangular and elliptic cross sections of different aspect ratios, for tubes of crescent-shaped cross sections, and a tube whose cross section is an oval of Cassini. For fully developed flow, results are compared with the corresponding exact