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Sample records for acoustic phonon dispersion

  1. Investigation of phononic crystals for dispersive surface acoustic wave ozone sensors

    NASA Astrophysics Data System (ADS)

    Westafer, Ryan S.

    The object of this research was to investigate dispersion in surface phononic crystals (PnCs) for application to a newly developed passive surface acoustic wave (SAW) ozone sensor. Frequency band gaps and slow sound already have been reported for PnC lattice structures. Such engineered structures are often advertised to reduce loss, increase sensitivity, and reduce device size. However, these advances have not yet been realized in the context of surface acoustic wave sensors. In early work, we computed SAW dispersion in patterned surface structures and we confirmed that our finite element computations of SAW dispersion in thin films and in one dimensional surface PnC structures agree with experimental results obtained by laser probe techniques. We analyzed the computations to guide device design in terms of sensitivity and joint spectral operating point. Next we conducted simulations and experiments to determine sensitivity and limit of detection for more conventional dispersive SAW devices and PnC sensors. Finally, we conducted extensive ozone detection trials on passive reflection mode SAW devices, using distinct components of the time dispersed response to compensate for the effect of temperature. The experimental work revealed that the devices may be used for dosimetry applications over periods of several days.

  2. Phonon dispersion in hypersonic two-dimensional phononic crystal membranes

    NASA Astrophysics Data System (ADS)

    Graczykowski, B.; Sledzinska, M.; Alzina, F.; Gomis-Bresco, J.; Reparaz, J. S.; Wagner, M. R.; Sotomayor Torres, C. M.

    2015-02-01

    We investigate experimentally and theoretically the acoustic phonon propagation in two-dimensional phononic crystal membranes. Solid-air and solid-solid phononic crystals were made of square lattices of holes and Au pillars in and on 250 nm thick single crystalline Si membrane, respectively. The hypersonic phonon dispersion was investigated using Brillouin light scattering. Volume reduction (holes) or mass loading (pillars) accompanied with second-order periodicity and local resonances are shown to significantly modify the propagation of thermally activated GHz phonons. We use numerical modeling based on the finite element method to analyze the experimental results and determine polarization, symmetry, or three-dimensional localization of observed modes.

  3. Functional crossover in the dispersion relations of magnons and phonons

    NASA Astrophysics Data System (ADS)

    Hoser, A.; Köbler, U.

    2016-09-01

    Experimental data are presented showing that the dispersion relations of magnons and acoustic phonons can consist of two sections with different functions of wave vector. In the low wave vector range a power function of wave vector often holds over a finite q-range while dispersions for larger wave vector values better approach the atomistic model predictions. In the magnon spectra ∼⃒qx power functions with exponents x=1.25, 1.5 and 2 are identified. The dispersion of the acoustic phonons can be a linear function of wave vector over a surprisingly large range of energy. Since the slope of the linear section agrees with the known sound velocities it can be concluded that the dispersion of the acoustic phonons has got attracted by the linear dispersion of the mass less Debye bosons (sound waves). Due to the different (translational) symmetries of bosons and atomistic excitations (magnons, phonons) the associated dispersions can attract each other. In the same way the different ∼⃒qx power functions in the magnon dispersions indicate that magnon dispersions are attracted by the dispersion of the bosons of the magnetic continuum (Goldstone bosons). This allows evaluation of the otherwise difficult to obtain dispersions of the Goldstone bosons from the known magnon dispersions. Interestingly, the dispersions of Goldstone bosons (Debye bosons) attract magnon dispersions (phonon dispersions) and not vice versa.

  4. Phonon dispersion relation of metallic glasses

    NASA Astrophysics Data System (ADS)

    Crespo, Daniel; Bruna, Pere; Valles, Araceli; Pineda, Eloi

    2016-10-01

    Experimental data on the phase sound speed of metallic glasses show anomalies in the terahertz range, reflecting an underlying complex behavior of their phonon dispersion spectrum not yet explained. We determine the phonon dispersion curve of metallic glasses by means of massive molecular dynamics simulations, allowing us to obtain the low-q region behavior with unprecedented detail. Results confirm that the sound speed is constant below the THz range, down to the macroscopic limit. On the contrary, a hardening of the sound speed, more notable in the transverse case, is found in the THz range. This behavior is modeled in terms of a relaxation model. The model gives quantitative agreement and allows us to determine a new threshold frequency ωh, at the end of the boson-peak region. Above ωh the shear modulus increases dramatically, reflecting the end of the amorphous-like acoustic propagation region characterized by the excess density of vibrational states.

  5. Acoustic phonon spectrum and thermal transport in nanoporous alumina arrays

    DOE PAGES

    Kargar, Fariborz; Ramirez, Sylvester; Debnath, Bishwajit; ...

    2015-10-28

    We report results of a combined investigation of thermal conductivity and acoustic phonon spectra in nanoporous alumina membranes with the pore diameter decreasing from D=180 nm to 25 nm. The samples with the hexagonally arranged pores were selected to have the same porosity Ø ≈13%. The Brillouin-Mandelstam spectroscopy measurements revealed bulk-like phonon spectrum in the samples with D = 180 nm pores and spectral features, which were attributed to spatial confinement, in the samples with 25 nm and 40 nm pores. The velocity of the longitudinal acoustic phonons was reduced in the samples with smaller pores. As a result, analysismore » of the experimental data and calculated phonon dispersion suggests that both phonon-boundary scattering and phonon spatial confinement affect heat conduction in membranes with the feature sizes D < 40 nm.« less

  6. Acoustic phonon spectrum and thermal transport in nanoporous alumina arrays

    SciTech Connect

    Kargar, Fariborz; Ramirez, Sylvester; Debnath, Bishwajit; Malekpour, Hoda; Lake, Roger; Balandin, Alexander A.

    2015-10-28

    We report results of a combined investigation of thermal conductivity and acoustic phonon spectra in nanoporous alumina membranes with the pore diameter decreasing from D=180 nm to 25 nm. The samples with the hexagonally arranged pores were selected to have the same porosity Ø ≈13%. The Brillouin-Mandelstam spectroscopy measurements revealed bulk-like phonon spectrum in the samples with D = 180 nm pores and spectral features, which were attributed to spatial confinement, in the samples with 25 nm and 40 nm pores. The velocity of the longitudinal acoustic phonons was reduced in the samples with smaller pores. As a result, analysis of the experimental data and calculated phonon dispersion suggests that both phonon-boundary scattering and phonon spatial confinement affect heat conduction in membranes with the feature sizes D < 40 nm.

  7. Acoustic superfocusing by solid phononic crystals

    SciTech Connect

    Zhou, Xiaoming; Assouar, M. Badreddine Oudich, Mourad

    2014-12-08

    We propose a solid phononic crystal lens capable of acoustic superfocusing beyond the diffraction limit. The unit cell of the crystal is formed by four rigid cylinders in a hosting material with a cavity arranged in the center. Theoretical studies reveal that the solid lens produces both negative refraction to focus propagating waves and surface states to amplify evanescent waves. Numerical analyses of the superfocusing effect of the considered solid phononic lens are presented with a separated source excitation to the lens. In this case, acoustic superfocusing beyond the diffraction limit is evidenced. Compared to the fluid phononic lenses, the solid lens is more suitable for ultrasonic imaging applications.

  8. Acoustic superfocusing by solid phononic crystals

    NASA Astrophysics Data System (ADS)

    Zhou, Xiaoming; Assouar, M. Badreddine; Oudich, Mourad

    2014-12-01

    We propose a solid phononic crystal lens capable of acoustic superfocusing beyond the diffraction limit. The unit cell of the crystal is formed by four rigid cylinders in a hosting material with a cavity arranged in the center. Theoretical studies reveal that the solid lens produces both negative refraction to focus propagating waves and surface states to amplify evanescent waves. Numerical analyses of the superfocusing effect of the considered solid phononic lens are presented with a separated source excitation to the lens. In this case, acoustic superfocusing beyond the diffraction limit is evidenced. Compared to the fluid phononic lenses, the solid lens is more suitable for ultrasonic imaging applications.

  9. Acoustic dispersive prism

    NASA Astrophysics Data System (ADS)

    Esfahlani, Hussein; Karkar, Sami; Lissek, Herve; Mosig, Juan R.

    2016-01-01

    The optical dispersive prism is a well-studied element, which allows separating white light into its constituent spectral colors, and stands in nature as water droplets. In analogy to this definition, the acoustic dispersive prism should be an acoustic device with capability of splitting a broadband acoustic wave into its constituent Fourier components. However, due to the acoustical nature of materials as well as the design and fabrication difficulties, there is neither any natural acoustic counterpart of the optical prism, nor any artificial design reported so far exhibiting an equivalent acoustic behaviour. Here, based on exotic properties of the acoustic transmission-line metamaterials and exploiting unique physical behaviour of acoustic leaky-wave radiation, we report the first acoustic dispersive prism, effective within the audible frequency range 800 Hz–1300 Hz. The dispersive nature, and consequently the frequency-dependent refractive index of the metamaterial are exploited to split the sound waves towards different and frequency-dependent directions. Meanwhile, the leaky-wave nature of the structure facilitates the sound wave radiation into the ambient medium.

  10. Acoustic dispersive prism.

    PubMed

    Esfahlani, Hussein; Karkar, Sami; Lissek, Herve; Mosig, Juan R

    2016-01-07

    The optical dispersive prism is a well-studied element, which allows separating white light into its constituent spectral colors, and stands in nature as water droplets. In analogy to this definition, the acoustic dispersive prism should be an acoustic device with capability of splitting a broadband acoustic wave into its constituent Fourier components. However, due to the acoustical nature of materials as well as the design and fabrication difficulties, there is neither any natural acoustic counterpart of the optical prism, nor any artificial design reported so far exhibiting an equivalent acoustic behaviour. Here, based on exotic properties of the acoustic transmission-line metamaterials and exploiting unique physical behaviour of acoustic leaky-wave radiation, we report the first acoustic dispersive prism, effective within the audible frequency range 800 Hz-1300 Hz. The dispersive nature, and consequently the frequency-dependent refractive index of the metamaterial are exploited to split the sound waves towards different and frequency-dependent directions. Meanwhile, the leaky-wave nature of the structure facilitates the sound wave radiation into the ambient medium.

  11. Acoustic dispersive prism

    PubMed Central

    Esfahlani, Hussein; Karkar, Sami; Lissek, Herve; Mosig, Juan R.

    2016-01-01

    The optical dispersive prism is a well-studied element, which allows separating white light into its constituent spectral colors, and stands in nature as water droplets. In analogy to this definition, the acoustic dispersive prism should be an acoustic device with capability of splitting a broadband acoustic wave into its constituent Fourier components. However, due to the acoustical nature of materials as well as the design and fabrication difficulties, there is neither any natural acoustic counterpart of the optical prism, nor any artificial design reported so far exhibiting an equivalent acoustic behaviour. Here, based on exotic properties of the acoustic transmission-line metamaterials and exploiting unique physical behaviour of acoustic leaky-wave radiation, we report the first acoustic dispersive prism, effective within the audible frequency range 800 Hz–1300 Hz. The dispersive nature, and consequently the frequency-dependent refractive index of the metamaterial are exploited to split the sound waves towards different and frequency-dependent directions. Meanwhile, the leaky-wave nature of the structure facilitates the sound wave radiation into the ambient medium. PMID:26739504

  12. Depth-Dependent Defect Studies Using Coherent Acoustic Phonons

    DTIC Science & Technology

    2014-09-29

    12211 Research Triangle Park, NC 27709-2211 coherent acoustic phonons, diamond, silicon, photelastic coefficients , refractive index, graphene, Second...attributed to the cooling of the subsystem of hot optical phonons by optical- acoustic phonon scattering . We observe that at different pump energy and...SECURITY CLASSIFICATION OF: Presented is our scientific progress in two areas of research. The first is coherent acoustic phonon (CAP) spectroscopy of

  13. Dispersive Phonon Imaging in Iii-V Semiconductors.

    NASA Astrophysics Data System (ADS)

    Hebboul, Saad Eddine

    Low-temperature transport properties of high-frequency acoustic phonons are investigated in GaAs, InSb, InP and InAs using the phonon-imaging technique. In this method, a focused laser beam provides a movable heat source on one side of a cooled crystal (<=q2 K). A single small phonon detector on the opposite face records the transmitted heat flux as a function of propagation direction. Ballistic phonons channel along directions in the crystal which are completely determined by the detailed shape of constant-energy surfaces in wavevector space. The resulting focusing patterns are characterized by sharp phonon caustics which are clearly identified from the continuous background due to scattered phonons. In the dispersive regime, where phonon wavelength is comparable to atomic spacing, the angular positions of these caustic lines are very sensitive to phonon frequency, thus providing a novel test for lattice dynamics theories. Experiments are performed with superconducting tunnel junctions and Al bolometers to probe both the high-frequency and low -frequency regimes, respectively. We find that large-k ballistic phonons give rise to distinct focusing patterns in all four types of crystals, with thicknesses varying between 0.4 and 0.8 mm. Due to isotope scattering in the bulk, tunnel-junction experiments yield well-defined caustic patterns with a dominant frequency given by the detector gap 2Delta. In InSb, where zone boundary frequencies are small (nu_ {TA} ~ 1.2 THz), the frequency dependence of the dispersive phonon focusing patterns are measured using PbTl (0.43, 0.59 THz) and PbBi (0.69, 0.73, 0.78, 0.82 THz) tunnel junction detectors. The results are interpreted with Monte Carlo calculations based on rigid, dipole, shell, and bond-charge models. Although each model yields satisfactory fits to the previously measured dispersion curves, the predicted patterns show remarkable differences in the caustic structures. This result underscores the utility of phonon imaging

  14. Calculating the Phonon Dispersion From First Principles

    NASA Astrophysics Data System (ADS)

    Ceballos, Frank; O'Hara, Andy; Slepko, Alexander; Demkov, Alexander

    2011-10-01

    The goal of this project was to construct a user-friendly tool that can compute the phonon dispersion for any solid with a periodic crystal structure. The phonon dispersion describes the crystal's vibrational properties and thermodynamic properties of the solid. Using the Vienna Ab-initio Simulation Package (VASP) we compute the forces between the atoms. Assuming harmonic approximation we numerically evaluate force constant matrix. The lattice Fourier transform of the force constants yields the dynamical matrix, whose eigenvalues and eigenvectors represent the allowed phonon frequencies and displacement patterns for specific k-vectors. Our code then plots the frequencies along high symmetry lines in the Brillouin zone. We will present our results for silicon, GaAs and ZrO2.

  15. Polaron action for multimode dispersive phonon systems

    NASA Astrophysics Data System (ADS)

    Kornilovitch, P. E.

    2006-03-01

    The path-integral approach to the tight-binding polaron is extended to multiple optical phonon modes of arbitrary dispersion and polarization. The nonlinear lattice effects are neglected. Only one electron band is considered. The electron-phonon interaction is of the density-displacement type, but can be of arbitrary spatial range and shape. Feynman’s analytical integration of ion trajectories is performed by transforming the electron-ion forces to the basis in which the phonon dynamical matrix is diagonal. The resulting polaron action is derived for the periodic and shifted boundary conditions in imaginary time. The former can be used for calculating polaron thermodynamics while the latter for the polaron mass and spectrum. The developed formalism is the analytical basis for numerical analysis of such models by path-integral Monte Carlo methods.

  16. Acoustic waves switch based on meta-fluid phononic crystals

    NASA Astrophysics Data System (ADS)

    Zhu, Xue-Feng

    2012-08-01

    The acoustic waves switch based on meta-fluid phononic crystals (MEFL PCs) is theoretically investigated. The MEFL PCs consist of fluid matrix and fluid-like inclusions with extremely anisotropic-density. The dispersion relations are calculated via the plane wave expansion method, which are in good agreement with the transmitted sound pressure level spectra obtained by the finite element method. The results show that the width of absolute band gap in MEFL PCs depends sensitively upon the orientation of the extremely anisotropic-density inclusions and reaches maximum at the rotating angle of 45°, with the gap position nearly unchanged. Also, the inter-mode conversion inside anisotropic-density inclusions can be ignored due to large acoustic mismatch. The study gives a possibility to realize greater flexibility and stronger effects in tuning the acoustic band gaps, which is very significant in the enhanced control over sound waves and has potential applications in ultrasonic imaging and therapy.

  17. Acoustic phonon propagation in ultra-thin Si membranes under biaxial stress field

    NASA Astrophysics Data System (ADS)

    Graczykowski, B.; Gomis-Bresco, J.; Alzina, F.; Reparaz, J. S.; Shchepetov, A.; Prunnila, M.; Ahopelto, J.; Sotomayor Torres, C. M.

    2014-07-01

    We report on stress induced changes in the dispersion relations of acoustic phonons propagating in 27 nm thick single crystalline Si membranes. The static tensile stress (up to 0.3 GPa) acting on the Si membranes was achieved using an additional strain compensating silicon nitride frame. Dispersion relations of thermally activated hypersonic phonons were measured by means of Brillouin light scattering spectroscopy. The theory of Lamb wave propagation is developed for anisotropic materials subjected to an external static stress field. The dispersion relations were calculated using the elastic continuum approximation and taking into account the acousto-elastic effect. We find an excellent agreement between the theoretical and the experimental dispersion relations.

  18. Monolithic phononic crystals with a surface acoustic band gap from surface phonon-polariton coupling.

    PubMed

    Yudistira, D; Boes, A; Djafari-Rouhani, B; Pennec, Y; Yeo, L Y; Mitchell, A; Friend, J R

    2014-11-21

    We theoretically and experimentally demonstrate the existence of complete surface acoustic wave band gaps in surface phonon-polariton phononic crystals, in a completely monolithic structure formed from a two-dimensional honeycomb array of hexagonal shape domain-inverted inclusions in single crystal piezoelectric Z-cut lithium niobate. The band gaps appear at a frequency of about twice the Bragg band gap at the center of the Brillouin zone, formed through phonon-polariton coupling. The structure is mechanically, electromagnetically, and topographically homogeneous, without any physical alteration of the surface, offering an ideal platform for many acoustic wave applications for photonics, phononics, and microfluidics.

  19. Phononic glass: a robust acoustic-absorption material.

    PubMed

    Jiang, Heng; Wang, Yuren

    2012-08-01

    In order to achieve strong wide band acoustic absorption under high hydrostatic pressure, an interpenetrating network structure is introduced into the locally resonant phononic crystal to fabricate a type of phononic composite material called "phononic glass." Underwater acoustic absorption coefficient measurements show that the material owns high underwater sound absorption coefficients over 0.9 in 12-30 kHz. Moreover, the quasi-static compressive behavior shows that the phononic glass has a compressive strength over 5 MPa which is crucial for underwater applications.

  20. Direct observation of confined acoustic phonon polarization branches in free-standing semiconductor nanowires

    PubMed Central

    Kargar, Fariborz; Debnath, Bishwajit; Kakko, Joona-Pekko; Säynätjoki, Antti; Lipsanen, Harri; Nika, Denis L.; Lake, Roger K.; Balandin, Alexander A.

    2016-01-01

    Similar to electron waves, the phonon states in semiconductors can undergo changes induced by external boundaries. However, despite strong scientific and practical importance, conclusive experimental evidence of confined acoustic phonon polarization branches in individual free-standing nanostructures is lacking. Here we report results of Brillouin—Mandelstam light scattering spectroscopy, which reveal multiple (up to ten) confined acoustic phonon polarization branches in GaAs nanowires with a diameter as large as 128 nm, at a length scale that exceeds the grey phonon mean-free path in this material by almost an order-of-magnitude. The dispersion modification and energy scaling with diameter in individual nanowires are in excellent agreement with theory. The phonon confinement effects result in a decrease in the phonon group velocity along the nanowire axis and changes in the phonon density of states. The obtained results can lead to more efficient nanoscale control of acoustic phonons, with benefits for nanoelectronic, thermoelectric and spintronic devices. PMID:27830698

  1. Acoustic phonons, surface plasmons and surface acoustic plasmons in a superlattice and their nonreciprocal device applications

    NASA Astrophysics Data System (ADS)

    Derov, John S.

    1987-05-01

    The literature was surveyed to determine potential applications of acoustic and plasma phenomena in superlattices. The use of folded zone acoustic phonons and acoustic surface plasmons in 3 to 5 compounds like AlGaAs/GaAs superlattices is addressed. A dielectric phonon filter is presented and an acoustic resonator is considered. Surface plasmons and surface acoustic plasmons are discussed and a transducer, delay line and mixer are proposed as applications. A 500 GHz isolator utilizing surface magnetoplasmons is also presented.

  2. ACOUSTIC RECTIFICATION IN DISPERSIVE MEDIA

    SciTech Connect

    Cantrell, John H.

    2009-03-03

    It is shown that the shapes of acoustic radiation-induced static strain and displacement pulses (rectified acoustic pulses) are defined locally by the energy density of the generating waveform. Dispersive properties are introduced analytically by assuming that the rectified pulses are functionally dependent on a phase factor that includes both dispersive and nonlinear terms. The dispersion causes an evolutionary change in the shape of the energy density profile that leads to the generation of solitons experimentally observed in fused silica.

  3. Single Circuit Parallel Computing with Phonons through Magneto-acoustics

    NASA Astrophysics Data System (ADS)

    Sklan, Sophia; Grossman, Jeffrey

    2013-03-01

    Phononic computing - the use of (typically thermal) vibrations for information processing - is a nascent technology; its capabilities are still being discovered. We analyze an alternative form of phononic computing inspired by optical, rather than electronic, computing. Using the acoustic Faraday effect, we design a phonon gyrator and thereby a means of performing computation through the manipulation of polarization in transverse phonon currents. Moreover, we establish that our gyrators act as generalized transistors and can construct digital logic gates. Exploiting the wave nature of phonons and the similarity of our logic gates, we demonstrate parallel computation within a single circuit, an effect presently unique to phonons. Finally, a generic method of designing these parallel circuits is introduced and used to analyze the feasibility of magneto-acoustic materials in realizing these circuits. This material is based upon work supported by the National Science Foundation Graduate Research Fellowship under Grant No. 1122374.

  4. Acoustic Bloch oscillations in a two-dimensional phononic crystal

    NASA Astrophysics Data System (ADS)

    He, Zhaojian; Peng, Shasha; Cai, Feiyan; Ke, Manzhu; Liu, Zhengyou

    2007-11-01

    We report the observation of acoustic Bloch oscillations at megahertz frequency in a two-dimensional phononic crystal. By creating periodically arrayed cavities with a decreasing gradient in width along one direction in the phononic crystal, acoustic Wannier-Stark ladders are created in the frequency domain. The oscillatory motion of an incident Gaussian pulse inside the sample is demonstrated by both simulation and experiment.

  5. Dispersion and absorption in one-dimensional nonlinear lattices: A resonance phonon approach

    NASA Astrophysics Data System (ADS)

    Xu, Lubo; Wang, Lei

    2016-09-01

    Based on the linear response theory, we propose a resonance phonon (r-ph) approach to study the renormalized phonons in a few one-dimensional nonlinear lattices. Compared with the existing anharmonic phonon (a-ph) approach, the dispersion relations derived from this approach agree with the expectations of the effective phonon (e-ph) theory much better. The application is also largely extended, i.e., it is applicable in many extreme situations, e.g., high frequency, high temperature, etc., where the existing one can hardly work. Furthermore, two separated phonon branches (one acoustic and one optical) with a clear gap in between can be observed by the r-ph approach in a diatomic anharmonic lattice. While only one combined branch can be detected in the same lattice with both the a-ph approach and the e-ph theory.

  6. The phononic crystals: An unending quest for tailoring acoustics

    NASA Astrophysics Data System (ADS)

    Kushwaha, Manvir S.

    2016-07-01

    Periodicity (in time or space) is a part and parcel of every living being: one can see, hear and feel it. Everyday examples are locomotion, respiration and heart beat. The reinforced N-dimensional periodicity over two or more crystalline solids results in the so-called phononic band gap crystals. These can have dramatic consequences on the propagation of phonons, vibrations and sound. The fundamental physics of cleverly fabricated phononic crystals can offer a systematic route to realize the Anderson localization of sound and vibrations. As to the applications, the phononic crystals are envisaged to find ways in the architecture, acoustic waveguides, designing transducers, elastic/acoustic filters, noise control, ultrasonics, medical imaging and acoustic cloaking, to mention a few. This review focuses on the brief sketch of the progress made in the field that seems to have prospered even more than was originally imagined in the early nineties.

  7. Probing confined acoustic phonons in free standing small gold nanoparticles

    SciTech Connect

    Mankad, Venu; Jha, Prafulla K.; Ravindran, T. R.

    2013-02-21

    Polarized and depolarized spectra from gold (Au) nanoparticles of different sizes are investigated in the small size range, between 3 and 7 nm, using low frequency Raman spectroscopy. Acoustic vibrations of the free-standing Au nanoparticles are demonstrated with frequencies ranging from 5 to 35 cm{sup -1}, opening the way to the development of the acoustic resonators. A blue shift in the phonon peaks along with the broadening is observed with a decrease in particle size. Comparison of the measured frequencies with vibrational dynamics calculation and an examination as from the transmission electron microscopy results ascertain that the low frequency phonon modes are due to acoustic phonon quantization. Our results show that the observed low frequency Raman scattering originates from the spherical (l = 0) and quadrupolar (l = 2) vibrations of the spheroidal mode due to plasmon mediated acoustic vibrations in Au nanoparticles.

  8. Stimulated emission of phonons in an acoustic cavity

    NASA Astrophysics Data System (ADS)

    Tilstra, Lieuwe Gijsbert

    2001-10-01

    This thesis will present experiments on stimulated emission of phonons in dilute ruby following complete population inversion of the Zeeman-split E(2E) Kramers doublet by selective pulsed optical pumping into its upper component. The resulting phonon avalanches are detected by use of the R1 luminescence emanating from the inverted zone, located near the end face where the laser beam enters the crystal. The phonons appear to team up into a highly directional phonon beam. The phonon frequency is tunable from, say, 10-100 GHz via the magnetic field splitting of the doublet. Remarkably, the population of the lower doublet component, which is a measure of the number of phonons generated, evolves with a sequence of distinct steps. The time interval in between these steps equals 2L/v, corresponding to the time the phonons need to return to the inverted zone by reflection at the opposite end face at a distance L. The end faces of the ruby crystal thus form an acoustic cavity. The phonon beam passes the inverted zone repeatedly to be amplified further, in a manner similar to light in an optical laser. In other words, the basic ingredients for a phonon laser have been established.

  9. Acoustic phonon dynamics in strained cubic and hexagonal GaN/Al2O3 superlattices

    NASA Astrophysics Data System (ADS)

    Sesion, P. D., Jr.; Albuquerque, E. L.; Vasconcelos, M. S.; Mauriz, P. W.; Freire, V. N.

    2006-06-01

    We study the acoustic-phonon spectra in periodic and quasiperiodic (Fibonacci type) superlattices made up from III V nitride materials (GaN) intercalated by sapphire (Al2O3). Due to the misalignments between the sapphire and the GaN layers that can lead to threading dislocation densities as high as 108-1010 cm-1, and a significant lattice mismatch (~14%), the phonon dynamics is described beyond the continuum elastic model using coupled elastic and electromagnetic equations, stressing the importance of the piezoelectric polarization field in a strained condition. We use a transfer-matrix treatment to simplify the algebra, which would be otherwise quite complicated, allowing a neat analytical expressions for the phonon dispersion relation. Furthermore, a quantitative analysis of the localization and magnitude of the allowed band widths in the phonon's spectra, as well as their scale law and the parametric spectrum of singularities f(α), are presented and discussed.

  10. Slow light and slow acoustic phonons in optophononic resonators

    NASA Astrophysics Data System (ADS)

    Villafañe, V.; Soubelet, P.; Bruchhausen, A. E.; Lanzillotti-Kimura, N. D.; Jusserand, B.; Lemaître, A.; Fainstein, A.

    2016-11-01

    Slow and confined light have been exploited in optoelectronics to enhance light-matter interactions. Here we describe the GaAs/AlAs semiconductor microcavity as a device that, depending on the excitation conditions, either confines or slows down both light and optically generated acoustic phonons. The localization of photons and phonons in the same place of space amplifies optomechanical processes. Picosecond laser pulses are used to study through time-resolved reflectivity experiments the coupling between photons and both confined and slow acoustic phonons when the laser is tuned either with the cavity (confined) optical mode or with the stop-band edge (slow) optical modes. A model that fully takes into account the modified propagation of the acoustic phonons and light in these resonant structures is used to describe the laser detuning dependence of the coherently generated phonon spectra and amplitude under these different modes of laser excitation. We observe that confined light couples only to confined mechanical vibrations, while slow light can generate both confined and slow coherent vibrations. A strong enhancement of the optomechanical coupling using confined photons and vibrations, and also with properly designed slow photon and phonon modes, is demonstrated. The prospects for the use of these optoelectronic devices in confined and slow optomechanics are addressed.

  11. Strain induced modification in phonon dispersion curves of monolayer boron pnictides

    SciTech Connect

    Jha, Prafulla K. E-mail: prafullaj@yahoo.com; Soni, Himadri R.

    2014-01-14

    In the frame work of density functional theory, the biaxial strain induced phonon dispersion curves of monolayer boron pnictides (BX, X = N, P, As, and Sb) have been investigated. The electron-ion interactions have been modelled using ultrasoft pseudopotentials while exchange-correlation energies have been approximated by the method of local density approximation in the parameterization of Perdew-Zunger. The longitudinal and transverse acoustic phonon modes of boron pnictide sheets show linear dependency on wave vector k{sup →} while out of plane mode varies as k{sup 2}. The in-plane longitudinal and out of plane transverse optical modes in boron nitride displaying significant dispersion similar to graphene. We have analyzed the biaxial strain dependent behaviour of out of plane acoustic phonon mode which is linked to ripple for four BX sheets using a model equation with shell elasticity theory. The strain induces the hardening of this mode with tendency to become more linear with increase in strain percentage. The strain induced hardening of out of plane acoustic phonon mode indicates the absence of rippling in these compounds. Our band structure calculations for both unstrained and strained 2D h-BX are consistent with previous calculations.

  12. Superlensing effect for surface acoustic waves in a pillar-based phononic crystal with negative refractive index

    SciTech Connect

    Addouche, Mahmoud Al-Lethawe, Mohammed A. Choujaa, Abdelkrim Khelif, Abdelkrim

    2014-07-14

    We demonstrate super resolution imaging for surface acoustic waves using a phononic structure displaying negative refractive index. This phononic structure is made of a monolithic square lattice of cylindrical pillars standing on a semi-infinite medium. The pillars act as acoustic resonator and induce a surface propagating wave with unusual dispersion. We found, under specific geometrical parameters, one propagating mode that exhibits negative refraction effect with negative effective index close to −1. Furthermore, a flat lens with finite number of pillars is designed to allow the focusing of an acoustic point source into an image with a resolution of (λ)/3 , overcoming the Rayleigh diffraction limit.

  13. Boron arsenide phonon dispersion from inelastic x-ray scattering: Potential for ultrahigh thermal conductivity

    NASA Astrophysics Data System (ADS)

    Ma, Hao; Li, Chen; Tang, Shixiong; Yan, Jiaqiang; Alatas, Ahmet; Lindsay, Lucas; Sales, Brian C.; Tian, Zhiting

    2016-12-01

    Cubic boron arsenide (BAs) was predicted to have an exceptionally high thermal conductivity (k ) ˜2000 W m-1K-1 at room temperature, comparable to that of diamond, based on first-principles calculations. Subsequent experimental measurements, however, only obtained a k of ˜200 W m-1K-1 . To gain insight into this discrepancy, we measured phonon dispersion of single-crystal BAs along high symmetry directions using inelastic x-ray scattering and compared these with first-principles calculations. Based on the measured phonon dispersion, we have validated the theoretical prediction of a large frequency gap between acoustic and optical modes and bunching of acoustic branches, which were considered the main reasons for the predicted ultrahigh k . This supports its potential to be a super thermal conductor if very-high-quality single-crystal samples can be synthesized.

  14. Boron arsenide phonon dispersion from inelastic x-ray scattering: Potential for ultrahigh thermal conductivity

    DOE PAGES

    Ma, Hao; Li, Chen; Tang, Shixiong; ...

    2016-12-14

    Cubic boron arsenide (BAs) was predicted to have an exceptionally high thermal conductivity (k) ~2000 Wm-1K-1 at room temperature, comparable to that of diamond, based on first-principles calculations. Subsequent experimental measurements, however, only obtained a k of ~200 Wm-1K-1. To gain insight into this discrepancy, we measured phonon dispersion of single crystal BAs along high symmetry directions using inelastic x-ray scattering (IXS) and compared these with first-principles calculations. Based on the measured phonon dispersion, we have validated the theoretical prediction of a large frequency gap between acoustic and optical modes and bunching of acoustic branches, which were considered the mainmore » reasons for the predicted ultrahigh k. This supports its potential to be a super thermal conductor if very high-quality single crystal samples can be synthesized.« less

  15. Boron arsenide phonon dispersion from inelastic x-ray scattering: Potential for ultrahigh thermal conductivity

    SciTech Connect

    Ma, Hao; Li, Chen; Tang, Shixiong; Yan, Jiaqiang; Alatas, Ahmet; Lindsay, Lucas; Sales, Brian C.; Tian, Zhiting

    2016-12-14

    Cubic boron arsenide (BAs) was predicted to have an exceptionally high thermal conductivity (k) ~2000 Wm-1K-1 at room temperature, comparable to that of diamond, based on first-principles calculations. Subsequent experimental measurements, however, only obtained a k of ~200 Wm-1K-1. To gain insight into this discrepancy, we measured phonon dispersion of single crystal BAs along high symmetry directions using inelastic x-ray scattering (IXS) and compared these with first-principles calculations. Based on the measured phonon dispersion, we have validated the theoretical prediction of a large frequency gap between acoustic and optical modes and bunching of acoustic branches, which were considered the main reasons for the predicted ultrahigh k. This supports its potential to be a super thermal conductor if very high-quality single crystal samples can be synthesized.

  16. Phononic crystal structures for acoustically driven microfluidic manipulations.

    PubMed

    Wilson, Rab; Reboud, Julien; Bourquin, Yannyk; Neale, Steven L; Zhang, Yi; Cooper, Jonathan M

    2011-01-21

    The development of microfluidic systems is often constrained both by difficulties associated with the chip interconnection to other instruments and by limitations imposed by the mechanisms that can enable fluid movement and processing. Surface acoustic wave (SAW) devices have shown promise in allowing samples to be manipulated, although designing complex fluid operations involves using multiple electrode transducers. We now demonstrate a simple interface between a piezoelectric SAW device and a disposable microfluidic chip, patterned with phononic structures to control the acoustic wave propagation. The surface wave is coupled from the piezoelectric substrate into the disposable chip where it interacts with the phononic lattice. By implementing both a phononic filter and an acoustic waveguide, we illustrate the potential of the technique by demonstrating microcentrifugation for particle and cell concentration in microlitre droplets. We show for the first time that the interaction of the fluid within this metamaterial phononic lattice is dependent upon the frequency of the acoustic wave, providing a route to programme complex fluidic functions into a microchip (in much the same way, by analogy, that a holographic element would change the phase of a light wave in optical tweezers). A practical realisation of this involves the centrifugation of blood on the chip.

  17. Phonon Dispersion in Chiral Single-Wall Carbon Nanotubes

    NASA Astrophysics Data System (ADS)

    Mu, Weihua; Vamivakas, Anthony Nickolas; Fang, Yan; Wang, Bolin

    The method to obtain phonon dispersion of achiral single-wall carbon nanotubes (SWNTs) from 6×6 matrix proposed by Mahan and Jeon7 has been extended to chiral SWNTs. The number of calculated phonon modes of a chiral SWNT (10, 1) is much larger than that of a zigzag one (10, 0) because the number of atoms in the translational unit cell of chiral SWNT is larger than that of an achiral one even though they have relative similar radius. The possible application of our approach to other models with more phonon potential terms beyond Mahan and Jeon's model is discussed.

  18. Phonon dispersion in red mercuric iodide

    SciTech Connect

    Sim, H.; Chang, Y. ); James, R.B. )

    1994-02-15

    We present theoretical studies of phonon modes of undoped HgI[sub 2] in its red tetragonal form. A rigid-ion model including the Coulomb interaction is used which gives the best fit to the neutron scattering, infrared reflectivity, and Raman scattering data. The calculated sound velocities are also in accord with experiment.

  19. Propagation and localization of acoustic waves in Fibonacci phononic circuits

    NASA Astrophysics Data System (ADS)

    Aynaou, H.; El Boudouti, E. H.; Djafari-Rouhani, B.; Akjouj, A.; Velasco, V. R.

    2005-07-01

    A theoretical investigation is made of acoustic wave propagation in one-dimensional phononic bandgap structures made of slender tube loops pasted together with slender tubes of finite length according to a Fibonacci sequence. The band structure and transmission spectrum is studied for two particular cases. (i) Symmetric loop structures, which are shown to be equivalent to diameter-modulated slender tubes. In this case, it is found that besides the existence of extended and forbidden modes, some narrow frequency bands appear in the transmission spectra inside the gaps as defect modes. The spatial localization of the modes lying in the middle of the bands and at their edges is examined by means of the local density of states. The dependence of the bandgap structure on the slender tube diameters is presented. An analysis of the transmission phase time enables us to derive the group velocity as well as the density of states in these structures. In particular, the stop bands (localized modes) may give rise to unusual (strong normal) dispersion in the gaps, yielding fast (slow) group velocities above (below) the speed of sound. (ii) Asymmetric tube loop structures, where the loops play the role of resonators that may introduce transmission zeros and hence new gaps unnoticed in the case of simple diameter-modulated slender tubes. The Fibonacci scaling property has been checked for both cases (i) and (ii), and it holds for a periodicity of three or six depending on the nature of the substrates surrounding the structure.

  20. Role of acoustic phonons in frequency dependent electronic thermal conductivity of graphene

    NASA Astrophysics Data System (ADS)

    Bhalla, Pankaj

    2017-03-01

    We study the effect of the electron-phonon interaction on the finite frequency dependent electronic thermal conductivity of two dimensional graphene. We calculate it for various acoustic phonons present in graphene and characterized by different dispersion relations using the memory function approach. It is found that the electronic thermal conductivity κe (T) in the zero frequency limit follows different power law for the longitudinal/transverse and the flexural acoustic phonons. For the longitudinal/transverse phonons, κe (T) ∼T-1 at the low temperature and saturates at the high temperature. These signatures qualitatively agree with the results calculated by solving the Boltzmann equation analytically and numerically. Similarly, for the flexural phonons, we find that κe (T) shows T 1 / 2 law at the low temperature and then saturates at the high temperature. In the finite frequency regime, we observe that the real part of the electronic thermal conductivity, Re [κe (ω , T) ] follows ω-2 behavior at the low frequency and becomes frequency independent at the high frequency.

  1. Nonlinear Transport and Noise Properties of Acoustic Phonons

    NASA Astrophysics Data System (ADS)

    Walczak, Kamil

    We examine heat transport carried by acoustic phonons in molecular junctions composed of organic molecules coupled to two thermal baths of different temperatures. The phononic heat flux and its dynamical noise properties are analyzed within the scattering (Landauer) formalism with transmission probability function for acoustic phonons calculated within the method of atomistic Green's functions (AGF technique). The perturbative computational scheme is used to determine nonlinear corrections to phononic heat flux and its noise power spectral density with up to the second order terms with respect to temperature difference. Our results show the limited applicability of ballistic Fourier's law and fluctuation-dissipation theorem to heat transport in quantum systems. We also derive several noise-signal relations applicable to nanoscale heat flow carried by phonons, but valid for electrons as well. We also discuss the extension of the perturbative transport theory to higher order terms in order to address a huge variety of problems related to nonlinear thermal effects which may occur at nanoscale and at strongly non-equilibrium conditions with high-intensity heat fluxes. This work was supported by Pace University Start-up Grant.

  2. Acoustic phonon transmission spectra in piezoelectric AlN/GaN Fibonacci phononic crystals

    NASA Astrophysics Data System (ADS)

    Sesion, P. D., Jr.; Albuquerque, E. L.; Chesman, C.; Freire, V. N.

    2007-08-01

    We study the acoustic-phonon transmission spectra in periodic and quasiperiodic (Fibonacci type) superlattices made up from the III-V nitride materials AlN and GaN. The phonon dynamics is described by a coupled elastic and electromagnetic equations within the static field approximation model, stressing the importance of the piezoelectric polarization field in a strained condition. We use a transfer-matrix treatment to simplify the algebra, which would be otherwise quite complicated, allowing a neat analytical expressions for the phonon transmission coefficients. Numerical results, for the normal incidence case, show a strike self-similar pattern for both hexagonal (class 6 mm) and cubic symmetries crystalizations of the nitrides.

  3. High temperature phonon dispersion in graphene using classical molecular dynamics

    SciTech Connect

    Anees, P. Panigrahi, B. K.; Valsakumar, M. C.

    2014-04-24

    Phonon dispersion and phonon density of states of graphene are calculated using classical molecular dynamics simulations. In this method, the dynamical matrix is constructed based on linear response theory by computing the displacement of atoms during the simulations. The computed phonon dispersions show excellent agreement with experiments. The simulations are done in both NVT and NPT ensembles at 300 K and found that the LO/TO modes are getting hardened at the Γ point. The NPT ensemble simulations capture the anharmonicity of the crystal accurately and the hardening of LO/TO modes is more pronounced. We also found that at 300 K the C-C bond length reduces below the equilibrium value and the ZA bending mode frequency becomes imaginary close to Γ along K-Γ direction, which indicates instability of the flat 2D graphene sheets.

  4. Ultra-directional source of longitudinal acoustic waves based on a two-dimensional solid/solid phononic crystal

    SciTech Connect

    Morvan, B.; Tinel, A.; Sainidou, R.; Rembert, P.; Vasseur, J. O.; Hladky-Hennion, A.-C.; Swinteck, N.; Deymier, P. A.

    2014-12-07

    Phononic crystals (PC) can be used to control the dispersion properties of acoustic waves, which are essential to direct their propagation. We use a PC-based two-dimensional solid/solid composite to demonstrate experimentally and theoretically the spatial filtering of a monochromatic non-directional wave source and its emission in a surrounding water medium as an ultra-directional beam with narrow angular distribution. The phenomenon relies on square-shaped equifrequency contours (EFC) enabling self-collimation of acoustic waves within the phononic crystal. Additionally, the angular width of collimated beams is controlled via the EFC size-shrinking when increasing frequency.

  5. Temperature Dependence of Brillouin Light Scattering Spectra of Acoustic Phonons in Silicon

    NASA Astrophysics Data System (ADS)

    Somerville, Kevin; Klimovich, Nikita; An, Kyongmo; Sullivan, Sean; Weathers, Annie; Shi, Li; Li, Xiaoqin

    2015-03-01

    Thermal management represents an outstanding challenge in many areas of technology. Electrons, optical phonons, and acoustic phonons are often driven out of local equilibrium in electronic devices or during laser-material interaction processes. Interest in non-equilibrium transport processes has motivated the development of Raman spectroscopy as a local temperature sensor of optical phonons and intermediate frequency acoustic phonons, whereas Brillouin light scattering (BLS) has recently been explored as a temperature sensor of low-frequency acoustic phonons. Here, we report temperature dependent BLS spectra of silicon, with Raman spectra taken simultaneously for comparison. The origins of the observed temperature dependence of the BLS peak position, linewidth, and intensity are examined in order to evaluate their potential use as temperature sensors for acoustic phonons. We determine that the integrated BLS intensity can be used measure the temperature of specific acoustic phonon modes. This work is supported by National Science Foundation (NSF) Thermal Transport Processes Program under Grant CBET-1336968.

  6. Acoustic phonon lifetimes and thermal transport in free-standing and strained graphene.

    PubMed

    Bonini, Nicola; Garg, Jivtesh; Marzari, Nicola

    2012-06-13

    We use first-principles methods based on density functional perturbation theory to characterize the lifetimes of the acoustic phonon modes and their consequences on the thermal transport properties of graphene. We show that using a standard perturbative approach, the transverse and longitudinal acoustic phonons in free-standing graphene display finite lifetimes in the long-wavelength limit, making them ill-defined as elementary excitations in samples of dimensions larger than ∼1 μm. This behavior is entirely due to the presence of the quadratic dispersions for the out-of-plane phonon (ZA) flexural modes that appear in free-standing low-dimensional systems. Mechanical strain lifts this anomaly, and all phonons remain well-defined at any wavelength. Thermal transport is dominated by ZA modes, and the thermal conductivity is predicted to diverge with system size for any amount of strain. These findings highlight strain and sample size as key parameters in characterizing or engineering heat transport in graphene.

  7. Acoustic phonon modes in asymmetric AlxGa1-xN/GaN/AlyGa1-yN quantum wells

    NASA Astrophysics Data System (ADS)

    Zan, Y. H.; Ban, S. L.; Chai, Y. J.; Qu, Y.

    2017-02-01

    Using an elastic continuum model, the dispersion relations and phonon modes of propagating, confined, half space and interface acoustic phonons in asymmetric AlxGa1-xN/GaN/Al1-yGayN quantum wells (QWs) have been solved theoretically with the varieties of Al components x and y. Contrary to the previous conclusions, some regulations for the existence of the above different acoustic phonons are revealed as well as the transition conditions among these modes are also discussed. With increase of wave vectors, the dispersion relations split into several groups. Because the classification of these groups is related to the eigen frequencies of bulk materials forming QWs, phonon modes in these groups will be confined or propagating in different layers of QWs. Furthermore, the gradients of the dispersion relations' asymptotes are the velocities of longitudinal and the transverse acoustic phonons propagating in bulk materials in turns. The properties of the dispersion relations and their phonon modes are also analyzed in depth based on the cut-off conditions. By the changing of Al components x and y, the bottom of these groups will be modified to adjust eigen frequencies of AlxGa1-xN or Al1-yGayN layers. But the propagation properties of acoustic phonon modes will remain unchanged in each section.

  8. Acoustic phonons in chrysotile asbestos probed by high-resolution inelastic x-ray scattering

    SciTech Connect

    Mamontov, Eugene; Vakhrushev, S. B.; Kumzerov, Yu. A,; Alatas, A.

    2009-01-01

    Acoustic phonons in an individual, oriented fiber of chrysotile asbestos (chemical formula Mg{sub 3}Si{sub 2}O{sub 5}(OH){sub 4}) were observed at room temperature in the inelastic x-ray measurement with a very high (meV) resolution. The x-ray scattering vector was aligned along [1 0 0] direction of the reciprocal lattice, nearly parallel to the long axis of the fiber. The latter coincides with [1 0 0] direction of the direct lattice and the axes of the nano-channels. The data were analyzed using a damped harmonic oscillator model. Analysis of the phonon dispersion in the first Brillouin zone yielded the longitudinal sound velocity of (9200 {+-} 600) m/s.

  9. Magnetophonon oscillations caused by acoustic phonons in bulk conductors

    NASA Astrophysics Data System (ADS)

    Raichev, O. E.

    2016-09-01

    The interaction of electrons with acoustic phonons under a magnetic field leads to a remarkable kind of magnetophonon oscillation of transport coefficients, recently discovered in two-dimensional electron systems. The present study shows that similar oscillations exist in bulk conductors and provides a theory of this phenomenon for the case of spherical Fermi surfaces. The resonance peaks occur when the product of the Fermi surface diameter by the sound velocity is a multiple of the cyclotron frequency. Theoretical predictions may facilitate the experimental observation of the phenomenon.

  10. Numerical investigation of diffraction of acoustic waves by phononic crystals

    NASA Astrophysics Data System (ADS)

    Moiseyenko, Rayisa P.; Declercq, Nico F.; Laude, Vincent

    2012-05-01

    Diffraction as well as transmission of acoustic waves by two-dimensional phononic crystals (PCs) composed of steel rods in water are investigated in this paper. The finite element simulations were performed in order to compute pressure fields generated by a line source that are incident on a finite size PC. Such field maps are analyzed based on the complex band structure for the infinite periodic PC. Finite size computations indicate that the exponential decrease of the transmission at deaf frequencies is much stronger than that in Bragg band gaps.

  11. Origin of the "waterfall" effect in phonon dispersion of relaxor perovskites.

    PubMed

    Hlinka, J; Kamba, S; Petzelt, J; Kulda, J; Randall, C A; Zhang, S J

    2003-09-05

    We have undertaken an inelastic neutron scattering study of the perovskite relaxor ferroelectric Pb(Zn(1/3)Nb(2/3))O3 with 8% PbTiO3 (PZN-8%PT) in order to elucidate the origin of the previously reported unusual kink on the low frequency transverse phonon dispersion curve (known as the "waterfall effect"). We show that its position (q(wf)) depends on the choice of the Brillouin zone and that the relation of q(wf) to the size of the polar nanoregions is highly improbable. The waterfall phenomenon is explained in the framework of a simple model of coupled damped harmonic oscillators representing the acoustic and optic phonon branches.

  12. Inelastic x-ray scattering measurements of phonon dispersion and lifetimes in PbTe1-x Se x alloys

    NASA Astrophysics Data System (ADS)

    Tian, Zhiting; Li, Mingda; Ren, Zhensong; Ma, Hao; Alatas, Ahmet; Wilson, Stephen D.; Li, Ju

    2015-09-01

    PbTe1-x Se x alloys are of special interest to thermoelectric applications. Inelastic x-ray scattering determination of phonon dispersion and lifetimes along the high symmetry directions for PbTe1-x Se x alloys are presented. By comparing with calculated results based on the virtual crystal model calculations combined with ab initio density functional theory, the validity of virtual crystal model is evaluated. The results indicate that the virtual crystal model is overall a good assumption for phonon frequencies and group velocities despite the softening of transverse acoustic phonon modes along [1 1 1] direction, while the treatment of lifetimes warrants caution. In addition, phonons remain a good description of vibrational modes in PbTe1-x Se x alloys.

  13. Inelastic x-ray scattering measurements of phonon dispersion and lifetimes in PbTe1-x Se x alloys.

    PubMed

    Tian, Zhiting; Li, Mingda; Ren, Zhensong; Ma, Hao; Alatas, Ahmet; Wilson, Stephen D; Li, Ju

    2015-09-23

    PbTe1-x Se x alloys are of special interest to thermoelectric applications. Inelastic x-ray scattering determination of phonon dispersion and lifetimes along the high symmetry directions for PbTe1-x Se x alloys are presented. By comparing with calculated results based on the virtual crystal model calculations combined with ab initio density functional theory, the validity of virtual crystal model is evaluated. The results indicate that the virtual crystal model is overall a good assumption for phonon frequencies and group velocities despite the softening of transverse acoustic phonon modes along [1 1 1] direction, while the treatment of lifetimes warrants caution. In addition, phonons remain a good description of vibrational modes in PbTe1-x Se x alloys.

  14. Temperature dependence of Brillouin light scattering spectra of acoustic phonons in silicon

    SciTech Connect

    Olsson, Kevin S.; Klimovich, Nikita; An, Kyongmo; Sullivan, Sean; Weathers, Annie; Shi, Li E-mail: elaineli@physics.utexas.edu; Li, Xiaoqin E-mail: elaineli@physics.utexas.edu

    2015-02-02

    Electrons, optical phonons, and acoustic phonons are often driven out of local equilibrium in electronic devices or during laser-material interaction processes. The need for a better understanding of such non-equilibrium transport processes has motivated the development of Raman spectroscopy as a local temperature sensor of optical phonons and intermediate frequency acoustic phonons, whereas Brillouin light scattering (BLS) has recently been explored as a temperature sensor of low-frequency acoustic phonons. Here, we report the measured BLS spectra of silicon at different temperatures. The origins of the observed temperature dependence of the BLS peak position, linewidth, and intensity are examined in order to evaluate their potential use as temperature sensors for acoustic phonons.

  15. Temperature dependence of Brillouin light scattering spectra of acoustic phonons in silicon

    NASA Astrophysics Data System (ADS)

    Olsson, Kevin S.; Klimovich, Nikita; An, Kyongmo; Sullivan, Sean; Weathers, Annie; Shi, Li; Li, Xiaoqin

    2015-02-01

    Electrons, optical phonons, and acoustic phonons are often driven out of local equilibrium in electronic devices or during laser-material interaction processes. The need for a better understanding of such non-equilibrium transport processes has motivated the development of Raman spectroscopy as a local temperature sensor of optical phonons and intermediate frequency acoustic phonons, whereas Brillouin light scattering (BLS) has recently been explored as a temperature sensor of low-frequency acoustic phonons. Here, we report the measured BLS spectra of silicon at different temperatures. The origins of the observed temperature dependence of the BLS peak position, linewidth, and intensity are examined in order to evaluate their potential use as temperature sensors for acoustic phonons.

  16. Phonon dispersion relation in PbTiO3

    NASA Astrophysics Data System (ADS)

    Tomeno, Izumi; Fernandez-Baca, Jaime; Marty, Karol; Oka, Kunihiko; Tsunoda, Yorihiko

    2013-03-01

    The phonon dispersion relations for cubic PbTiO3 (Tc = 763 K) have been determined along the high symmetry directions at T = 793 K using inelastic neutron scattering. A set of the TO branches drops significantly toward the zone center. This is quite different from the soft mode anomaly in the Pb-based relaxors, named as the waterfall phenomenon. The zone-center TO mode energy softens with decreasing temperature from 1173 to 793 K. The TA branch along [ ξ , ξ , ξ ] shows significant softening around ξ = 0.25 and 0.5. These two anomalies persist up to 1173 K and are weakly temperature dependent. Moreover, the TA branches along [1,0,0] and [1,1,0] soften in the entire q range as the temperature approaches Tc. Although the phonon softening occurs simultaneously, the softening of the zone center TO mode plays an important role in the single phase transition. The phonon dispersion relations for cubic and tetragonal PbTiO3 are discussed in connection with BaTiO3, KTaO3, Pb(Zn1/3Nb2/3)O3, and Pb(Mg1/3Nb2/3)O3. U.S.-Japan cooperative program on neutron scattering

  17. Surface acoustic waves in two dimensional phononic crystal with anisotropic inclusions

    NASA Astrophysics Data System (ADS)

    Ketata, H.; Hédi Ben Ghozlen, M.

    2012-06-01

    An analysis is given to the band structure of the two dimensional solid phononic crystal considered as a semi infinite medium. The lattice includes an array of elastic anisotropic materials with different shapes embedded in a uniform matrix. For illustration two kinds of phononic materials are assumed. A particular attention is devoted to the computational procedure which is mainly based on the plane wave expansion (PWE) method. It has been adapted to Matlab environment. Numerical calculations of the dispersion curves have been achieved by introducing particular functions which transform motion equations into an Eigen value problem. Significant improvements are obtained by increasing reasonably the number of Fourier components even when a large elastic mismatch is assumed. Such approach can be generalized to different types of symmetry and permit new physical properties as piezoelectricity to be added. The actual semi infinite phononic structure with a free surface has been shown to support surface acoustic waves (SAW). The obtained dispersion curves reveal band gaps in the SAW branches. It has been found that the influence, of the filling factor and anisotropy on their band gaps, is different from that of bulk waves.

  18. Effect of electron heating on femtosecond laser-induced coherent acoustic phonons in noble metals

    NASA Astrophysics Data System (ADS)

    Wang, Jincheng; Guo, Chunlei

    2007-05-01

    We employ a surface plasmon technique to resolve the dynamics of femtosecond-laser-induced coherent acoustic phonons in noble metals. Clear acoustic oscillations are observed in our experiments. We further study the dependence of the initial phase of the oscillations on pump fluence, and we find that the initial phase decreases linearly with pump fluence. Our model calculations show that hot electrons instantaneously excited by femtosecond pulses contribute to the generation of coherent acoustic phonons in metals.

  19. Piezoelectric surface acoustical phonon amplification in graphene on a GaAs substrate

    SciTech Connect

    Nunes, O. A. C.

    2014-06-21

    We study the interaction of Dirac Fermions in monolayer graphene on a GaAs substrate in an applied electric field by the combined action of the extrinsic potential of piezoelectric surface acoustical phonons of GaAs (piezoelectric acoustical (PA)) and of the intrinsic deformation potential of acoustical phonons in graphene (deformation acoustical (DA)). We find that provided the dc field exceeds a threshold value, emission of piezoelectric (PA) and deformation (DA) acoustical phonons can be obtained in a wide frequency range up to terahertz at low and high temperatures. We found that the phonon amplification rate R{sup PA,DA} scales with T{sub BG}{sup S−1} (S=PA,DA), T{sub BG}{sup S} being the Block−Gru{sup ¨}neisen temperature. In the high-T Block−Gru{sup ¨}neisen regime, extrinsic PA phonon scattering is suppressed by intrinsic DA phonon scattering, where the ratio R{sup PA}/R{sup DA} scales with ≈1/√(n), n being the carrier concentration. We found that only for carrier concentration n≤10{sup 10}cm{sup −2}, R{sup PA}/R{sup DA}>1. In the low-T Block−Gru{sup ¨}neisen regime, and for n=10{sup 10}cm{sup −2}, the ratio R{sup PA}/R{sup DA} scales with T{sub BG}{sup DA}/T{sub BG}{sup PA}≈7.5 and R{sup PA}/R{sup DA}>1. In this regime, PA phonon dominates the electron scattering and R{sup PA}/R{sup DA}<1 otherwise. This study is relevant to the exploration of the acoustic properties of graphene and to the application of graphene as an acoustical phonon amplifier and a frequency-tunable acoustical phonon device.

  20. Ultralow frequency acoustic bandgap and vibration energy recovery in tetragonal folding beam phononic crystal

    NASA Astrophysics Data System (ADS)

    Gao, Nansha; Wu, Jiu Hui; Yu, Lie; Hou, Hong

    2016-06-01

    This paper investigates ultralow frequency acoustic properties and energy recovery of tetragonal folding beam phononic crystal (TFBPC) and its complementary structure. The dispersion curve relationships, transmission spectra and displacement fields of the eigenmodes are studied with FEA in detail. Compared with the traditional three layer phononic crystal (PC) structure, this structure proposed in this paper not only unfold bandgaps (BGs) in lower frequency range (below 300 Hz), but also has lighter weight because of beam structural cracks. We analyze the relevant physical mechanism behind this phenomenon, and discuss the effects of the tetragonal folding beam geometric parameters on band structure maps. FEM proves that the multi-cell structures with different arrangements have different acoustic BGs when compared with single cell structure. Harmonic frequency response and piezoelectric properties of TFBPC are specifically analyzed. The results confirm that this structure does have the recovery ability for low frequency vibration energy in environment. These conclusions in this paper could be indispensable to PC practical applications such as BG tuning and could be applied in portable devices, wireless sensor, micro-electro mechanical systems which can recycle energy from vibration environment as its own energy supply.

  1. Influence of confined acoustic phonons on the Radioelectric field in a Quantum well

    NASA Astrophysics Data System (ADS)

    Long, Do Tuan; Quang Bau, Nguyen

    2015-06-01

    The influence of confined acoustic phonons on the Radioelectric field in a quantum well has been studied in the presence of a linearly polarized electromagnetic wave and a laser radiation. By using the quantum kinetic equation for electrons with confined electrons - confined acoustic phonons interaction, the analytical expression for the Radio electric field is obtained. The formula of the Radio electric field contains the quantum number m characterizing the phonons confinement and comes back to the case of unconfined phonons when m reaches to zero. The dependence of the Radio electric field on the frequency of the laser radiation, in case of confined acoustic phonons, is also achieved by numerical method for a specific quantum well AlGaAs/GaAs/AlGaAs. Results show that the Radio electric field has a peak and reaches saturation as the frequency of the laser radiation increases.

  2. Waveform-preserved unidirectional acoustic transmission based on impedance-matched acoustic metasurface and phononic crystal

    NASA Astrophysics Data System (ADS)

    Song, Ai-Ling; Chen, Tian-Ning; Wang, Xiao-Peng; Wan, Le-Le

    2016-08-01

    The waveform distortion happens in most of the unidirectional acoustic transmission (UAT) devices proposed before. In this paper, a novel type of waveform-preserved UAT device composed of an impedance-matched acoustic metasurface (AMS) and a phononic crystal (PC) structure is proposed and numerically investigated. The acoustic pressure field distributions and transmittance are calculated by using the finite element method. The subwavelength AMS that can modulate the wavefront of the transmitted wave at will is designed and the band structure of the PC structure is calculated and analyzed. The sound pressure field distributions demonstrate that the unidirectional acoustic transmission can be realized by the proposed UAT device without changing the waveforms of the output waves, which is the distinctive feature compared with the previous UAT devices. The physical mechanism of the unidirectional acoustic transmission is discussed by analyzing the refraction angle changes and partial band gap map. The calculated transmission spectra show that the UAT device is valid within a relatively broad frequency range. The simulation results agree well with the theoretical predictions. The proposed UAT device provides a good reference for designing waveform-preserved UAT devices and has potential applications in many fields, such as medical ultrasound, acoustic rectifiers, and noise insulation.

  3. Dispersion properties of the phononic crystal consisting of ellipse-shaped particles

    NASA Astrophysics Data System (ADS)

    Pavlov, I. S.; Vasiliev, A. A.; Porubov, A. V.

    2016-12-01

    A two-dimensional model is considered in the form of a phononic crystal having a rectangular lattice with elastically interacting ellipse-shaped particles possessing two translational and one rotational degrees of freedom. The linear differential-difference equations are obtained by the method of structural modeling to describe propagation of longitudinal, transverse and rotational waves in the medium. It is found analytically how the coefficients of the equations depend on the sizes of the particle and on the parameters of interactions between them. The dispersion properties of the model are analyzed. Existence of a backward wave is established. The threshold frequencies of acoustic and rotational waves in some crystalline materials with cubic symmetry are estimated.

  4. Intermolecular electron transfer from intramolecular excitation and coherent acoustic phonon generation in a hydrogen-bonded charge-transfer solid

    NASA Astrophysics Data System (ADS)

    Rury, Aaron S.; Sorenson, Shayne; Dawlaty, Jahan M.

    2016-03-01

    Organic materials that produce coherent lattice phonon excitations in response to external stimuli may provide next generation solutions in a wide range of applications. However, for these materials to lead to functional devices in technology, a full understanding of the possible driving forces of coherent lattice phonon generation must be attained. To facilitate the achievement of this goal, we have undertaken an optical spectroscopic study of an organic charge-transfer material formed from the ubiquitous reduction-oxidation pair hydroquinone and p-benzoquinone. Upon pumping this material, known as quinhydrone, on its intermolecular charge transfer resonance as well as an intramolecular resonance of p-benzoquinone, we find sub-cm-1 oscillations whose dispersion with probe energy resembles that of a coherent acoustic phonon that we argue is coherently excited following changes in the electron density of quinhydrone. Using the dynamical information from these ultrafast pump-probe measurements, we find that the fastest process we can resolve does not change whether we pump quinhydrone at either energy. Electron-phonon coupling from both ultrafast coherent vibrational and steady-state resonance Raman spectroscopies allows us to determine that intramolecular electronic excitation of p-benzoquinone also drives the electron transfer process in quinhydrone. These results demonstrate the wide range of electronic excitations of the parent of molecules found in many functional organic materials that can drive coherent lattice phonon excitations useful for applications in electronics, photonics, and information technology.

  5. Envelope Solitons in Acoustically Dispersive Vitreous Silica

    NASA Technical Reports Server (NTRS)

    Cantrell, John H.; Yost, William T.

    2012-01-01

    Acoustic radiation-induced static strains, displacements, and stresses are manifested as rectified or dc waveforms linked to the energy density of an acoustic wave or vibrational mode via the mode nonlinearity parameter of the material. An analytical model is developed for acoustically dispersive media that predicts the evolution of the energy density of an initial waveform into a series of energy solitons that generates a corresponding series of radiation-induced static strains (envelope solitons). The evolutionary characteristics of the envelope solitons are confirmed experimentally in Suprasil W1 vitreous silica. The value (-11.9 plus or minus 1.43) for the nonlinearity parameter, determined from displacement measurements of the envelope solitons via a capacitive transducer, is in good agreement with the value (-11.6 plus or minus 1.16) obtained independently from acoustic harmonic generation measurements. The agreement provides strong, quantitative evidence for the validity of the model.

  6. Phonon dispersion and quantization tuning of strained carbon nanotubes for flexible electronics

    SciTech Connect

    Gautreau, Pierre; Chu, Yanbiao; Basaran, Cemal; Ragab, Tarek

    2014-06-28

    Graphene and carbon nanotubes are materials with large potentials for applications in flexible electronics. Such devices require a high level of sustainable strain and an understanding of the materials electrical properties under strain. Using supercell theory in conjunction with a comprehensive molecular mechanics model, the full band phonon dispersion of carbon nanotubes under uniaxial strain is studied. The results suggest an overall phonon softening and open up the possibility of phonon quantization tuning with uniaxial strain. The change in phonon quantization and the resulting increase in electron-phonon and phonon-phonon scattering rates offer further explanation and theoretical basis to the experimental observation of electrical properties degradation for carbon nanotubes under uniaxial strain.

  7. Interface nano-confined acoustic waves in polymeric surface phononic crystals

    SciTech Connect

    Travagliati, Marco; Nardi, Damiano; Giannetti, Claudio; Ferrini, Gabriele; Banfi, Francesco; Gusev, Vitalyi; Pingue, Pasqualantonio; Piazza, Vincenzo

    2015-01-12

    The impulsive acoustic dynamics of soft polymeric surface phononic crystals is investigated here in the hypersonic frequency range by near-IR time-resolved optical diffraction. The acoustic response is analysed by means of wavelet spectral methods and finite element modeling. An unprecedented class of acoustic modes propagating within the polymer surface phononic crystal and confined within 100 nm of the nano-patterned interface is revealed. The present finding opens the path to an alternative paradigm for characterizing the mechanical properties of soft polymers at interfaces and for sensing schemes exploiting polymers as embedding materials.

  8. Interface nano-confined acoustic waves in polymeric surface phononic crystals

    NASA Astrophysics Data System (ADS)

    Travagliati, Marco; Nardi, Damiano; Giannetti, Claudio; Gusev, Vitalyi; Pingue, Pasqualantonio; Piazza, Vincenzo; Ferrini, Gabriele; Banfi, Francesco

    2015-01-01

    The impulsive acoustic dynamics of soft polymeric surface phononic crystals is investigated here in the hypersonic frequency range by near-IR time-resolved optical diffraction. The acoustic response is analysed by means of wavelet spectral methods and finite element modeling. An unprecedented class of acoustic modes propagating within the polymer surface phononic crystal and confined within 100 nm of the nano-patterned interface is revealed. The present finding opens the path to an alternative paradigm for characterizing the mechanical properties of soft polymers at interfaces and for sensing schemes exploiting polymers as embedding materials.

  9. Bleustein-Gulyaev-Shimizu surface acoustic waves in two-dimensional piezoelectric phononic crystals.

    PubMed

    Hsu, Jin-Chen; Wu, Tsung-Tsong

    2006-06-01

    In this paper, we present a study on the existence of Bleustein-Gulyaev-Shimizu piezoelectric surface acoustic waves in a two-dimensional piezoelectric phononic crystal (zinc oxide, ZnO, and cadmium-sulfide, CdS) using the plane wave expansion method. In the configuration of ZnO (100)/CdS(100) phononic crystal, the calculated results show that this type of surface waves has higher acoustic wave velocities, high electromechanical coupling coefficients, and larger band gap width than those of the Rayleigh surface waves and pseudosurface waves. In addition, we find that the folded modes of the Bleustein-Gulyaev-Shimizu surface waves have higher coupling coefficients.

  10. Electron–acoustic phonon coupling in single crystal CH3NH3PbI3 perovskites revealed by coherent acoustic phonons

    PubMed Central

    Mante, Pierre-Adrien; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.; Yartsev, Arkady

    2017-01-01

    Despite the great amount of attention CH3NH3PbI3 has received for its solar cell application, intrinsic properties of this material are still largely unknown. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. We apply this method to characterize a CH3NH3PbI3 single crystal. We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using the deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. Our results reveal high electron and hole mobilities of 2,800 and 9,400 cm2 V−1 s−1, respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3. PMID:28176755

  11. Electron-acoustic phonon coupling in single crystal CH3NH3PbI3 perovskites revealed by coherent acoustic phonons.

    PubMed

    Mante, Pierre-Adrien; Stoumpos, Constantinos C; Kanatzidis, Mercouri G; Yartsev, Arkady

    2017-02-08

    Despite the great amount of attention CH3NH3PbI3 has received for its solar cell application, intrinsic properties of this material are still largely unknown. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. We apply this method to characterize a CH3NH3PbI3 single crystal. We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using the deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. Our results reveal high electron and hole mobilities of 2,800 and 9,400 cm(2) V(-1) s(-1), respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3.

  12. Electron–acoustic phonon coupling in single crystal CH3NH3PbI3 perovskites revealed by coherent acoustic phonons

    DOE PAGES

    Mante, Pierre-Adrien; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.; ...

    2017-02-08

    The intrinsic properties of CH3NH3PbI3 are still largely unknown in spite of the great amount of attention it has received for its solar cell application. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. Furthermore, we apply this method to characterize a CH3NH3PbI3 single crystal.We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using themore » deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. These results reveal high electron and hole mobilities of 2,800 and 9,400 cm2V-1 s -1 , respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3.« less

  13. Electron-acoustic phonon coupling in single crystal CH3NH3PbI3 perovskites revealed by coherent acoustic phonons

    NASA Astrophysics Data System (ADS)

    Mante, Pierre-Adrien; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.; Yartsev, Arkady

    2017-02-01

    Despite the great amount of attention CH3NH3PbI3 has received for its solar cell application, intrinsic properties of this material are still largely unknown. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. We apply this method to characterize a CH3NH3PbI3 single crystal. We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using the deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. Our results reveal high electron and hole mobilities of 2,800 and 9,400 cm2 V-1 s-1, respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3.

  14. Acoustic beam splitting at low GHz frequencies in a defect-free phononic crystal

    NASA Astrophysics Data System (ADS)

    Guo, Yuning; Brick, Delia; Großmann, Martin; Hettich, Mike; Dekorsy, Thomas

    2017-01-01

    The directional waveguiding in a 2D phononic crystal is simulated based on the analysis of equifrequency contours. This approach is utilized to investigate acoustic beam splitting in a defect-free nanostructure in the low GHz range. We find relaxed limitations regarding the source parameters compared to similar approaches in the sonic regime. Finally, we discuss the possibility to design an acoustic interferometer device at the nanoscale at GHz frequencies.

  15. Acoustic phonon dynamics in thin-films of the topological insulator Bi2Se3

    NASA Astrophysics Data System (ADS)

    Glinka, Yuri D.; Babakiray, Sercan; Johnson, Trent A.; Holcomb, Mikel B.; Lederman, David

    2015-04-01

    Transient reflectivity traces measured for nanometer-sized films (6-40 nm) of the topological insulator Bi2Se3 revealed GHz-range oscillations driven within the relaxation of hot carriers photoexcited with ultrashort (˜100 fs) laser pulses of 1.51 eV photon energy. These oscillations have been suggested to result from acoustic phonon dynamics, including coherent longitudinal acoustic phonons in the form of standing acoustic waves. An increase of oscillation frequency from ˜35 to ˜70 GHz with decreasing film thickness from 40 to 15 nm was attributed to the interplay between two different regimes employing traveling-acoustic-waves for films thicker than 40 nm and the film bulk acoustic wave resonator (FBAWR) modes for films thinner than 40 nm. The amplitude of oscillations decays rapidly for films below 15 nm thick when the indirect intersurface coupling in Bi2Se3 films switches the FBAWR regime to that of the Lamb wave excitation. The frequency range of coherent longitudinal acoustic phonons is in good agreement with elastic properties of Bi2Se3.

  16. Dexterous acoustic trapping and patterning of particles assisted by phononic crystal plate

    SciTech Connect

    Wang, Tian; Ke, Manzhu Xu, Shengjun; Feng, Junheng; Qiu, Chunyin; Liu, Zhengyou

    2015-04-20

    In this letter, we present experimental demonstration of multi-particles trapping and patterning by the artificially engineered acoustic field of phononic crystal plate. Polystyrene particles are precisely trapped and patterned in two dimensional arrays, for example, the square, triangular, or quasi-periodic arrays, depending on the structures of the phononic crystal plates with varying sub-wavelength holes array. Analysis shows that the enhanced acoustic radiation force, induced by the resonant transmission field highly localized near the sub-wavelength apertures, accounts for the particles self-organizing. It can be envisaged that this kind of simple design of phononic crystal plates would pave an alternative route for self-assembly of particles and may be utilized in the lab-on-a-chip devices.

  17. Observation of induced longitudinal and shear acoustic phonons by Brillouin scattering.

    PubMed

    Yoshida, Taisuke; Matsukawa, Mami; Yanagitani, Takahiko

    2011-06-01

    To improve the accuracy of velocity measurements in the Brillouin scattering technique using weak thermal phonons, we have used induced coherent phonons, which intensify the scattering. To induce phonons in the gigahertz range, we used a c-axis tilted ZnO film transducer that was developed in our laboratory. This allowed us to induce longitudinal and shear acoustic phonons effectively at hypersonic frequencies. As a result, we obtained scattered light in the silica glass sample that was much more intense than that obtained from the thermal phonons. Because the Brillouin scattering from induced phonons was measured, the shift frequency was that of the electric signal applied to the ZnO transducer. Strong peaks lead to a reduction of the measurement time. This is useful for two-dimensional mapping of thin film elasticity using Brillouin scattering. Additionally, Brillouin scattering enables the simultaneous measurement of longitudinal and shear phonon velocities in the sample plane. This opens up a potential new technique for non-destructive elasticity measurements of various materials.

  18. Surface-phonon dispersion of a NiO(100) thin film

    NASA Astrophysics Data System (ADS)

    Kostov, K. L.; Polzin, S.; Saha, S. K.; Brovko, O.; Stepanyuk, V.; Widdra, W.

    2013-06-01

    A well-ordered 25 ML epitaxial NiO(100) film on Ag(100) as prepared by layer-by-layer growth has been characterized by high-resolution electron energy loss spectroscopy. Six different phonon branches have been identified in the Γ¯X¯ direction of the surface Brillouin zone and are compared with first-principles phonon calculations. Whereas the surface Rayleigh mode shows a strong upward dispersion of 173 cm-1 in agreement with observations for the NiO(100) single crystal, the other surface phonons and surface resonances show only smaller dispersion widths in Γ¯X¯ direction. The Wallis and the Lucas phonons are localized at 425 and 367 cm-1 at the Γ¯ point, respectively. Additionally, two phonons are identified that have stronger weight at the zone boundary at 194 and 285 cm-1 and that become surface resonances at the zone center. The dominant spectral feature is the Fuchs-Kliewer (FK) phonon polariton at 559 cm-1, which is excited by dipole scattering and exhibits a rather broad non-Lorentzian lineshape. The lineshape is explained by a FK splitting resulting from the splitting of bulk optical phonons due to antiferromagnetic order. This view is supported by calculations of the surface-loss function from bulk reflectivity data.

  19. Design of acoustic beam aperture modifier using gradient-index phononic crystals

    NASA Astrophysics Data System (ADS)

    Lin, Sz-Chin Steven; Tittmann, Bernhard R.; Huang, Tony Jun

    2012-06-01

    This article reports the design concept of a novel acoustic beam aperture modifier using butt-jointed gradient-index phononic crystals (GRIN PCs) consisting of steel cylinders embedded in a homogeneous epoxy background. By gradually tuning the period of a GRIN PC, the propagating direction of acoustic waves can be continuously bent to follow a sinusoidal trajectory in the structure. The aperture of an acoustic beam can therefore be shrunk or expanded through change of the gradient refractive index profiles of the butt-jointed GRIN PCs. Our computational results elucidate the effectiveness of the proposed acoustic beam aperture modifier. Such an acoustic device can be fabricated through a simple process and will be valuable in applications, such as biomedical imaging and surgery, nondestructive evaluation, communication, and acoustic absorbers.

  20. Multi-resonance tunneling of acoustic waves in two-dimensional locally-resonant phononic crystals

    NASA Astrophysics Data System (ADS)

    Yang, Aichao; He, Wei; Zhang, Jitao; Zhu, Liang; Yu, Lingang; Ma, Jian; Zou, Yang; Li, Min; Wu, Yu

    2017-03-01

    Multi-resonance tunneling of acoustic waves through a two-dimensional phononic crystal (PC) is demonstrated by substituting dual Helmholtz resonators (DHRs) for acoustically-rigid scatterers in the PC. Due to the coupling of the incident waves with the acoustic multi-resonance modes of the DHRs, acoustic waves can tunnel through the PC at specific frequencies which lie inside the band gaps of the PC. This wave tunneling transmission can be further broadened by using the multilayer Helmholtz resonators. Thus, a PC consisting of an array of dual/multilayer Helmholtz resonators can serve as an acoustic band-pass filter, used to pick out acoustic waves with certain frequencies from noise.

  1. Sub-Poissonian phonon statistics in an acoustical resonator coupled to a pumped two-level emitter

    NASA Astrophysics Data System (ADS)

    Ceban, V.; Macovei, M. A.

    2015-11-01

    The concept of an acoustical analog of the optical laser has been developed recently in both theoretical and experimental works. We here discuss a model of a coherent phonon generator with a direct signature of the quantum properties of sound vibrations. The considered setup is made of a laser-driven quantum dot embedded in an acoustical nanocavity. The system dynamics is solved for a single phonon mode in the steady-state and in the strong quantum dot—phonon coupling regime beyond the secular approximation. We demonstrate that the phonon statistics exhibits quantum features, i.e., is sub-Poissonian.

  2. Sub-Poissonian phonon statistics in an acoustical resonator coupled to a pumped two-level emitter

    SciTech Connect

    Ceban, V. Macovei, M. A.

    2015-11-15

    The concept of an acoustical analog of the optical laser has been developed recently in both theoretical and experimental works. We here discuss a model of a coherent phonon generator with a direct signature of the quantum properties of sound vibrations. The considered setup is made of a laser-driven quantum dot embedded in an acoustical nanocavity. The system dynamics is solved for a single phonon mode in the steady-state and in the strong quantum dot—phonon coupling regime beyond the secular approximation. We demonstrate that the phonon statistics exhibits quantum features, i.e., is sub-Poissonian.

  3. Peculiar transmission property of acoustic waves in a one-dimensional layered phononic crystal

    NASA Astrophysics Data System (ADS)

    Zhao, Degang; Wang, Wengang; Liu, Zhengyou; Shi, Jing; Wen, Weijia

    2007-03-01

    In this article, we report both theoretical calculation and experimental observation of acoustic waves abnormally through a one-dimensional layered transmitted phononic crystal at frequencies within the band gap into a material of large acoustic impedance mismatch, with an efficiency as high as unity. The transmission peaks can be interpreted as a result of the interference of acoustic waves reflected from all periodically aligned interfaces. The condition for the appearance of peaks is analyzed in detail and the optimized layer number is given for different configurations.

  4. Low-energy phonon dispersion in LaFe4Sb12

    NASA Astrophysics Data System (ADS)

    Leithe-Jasper, Andreas; Boehm, Martin; Mutka, Hannu; Koza, Michael M.

    We studied the vibrational dynamics of a single crystal of LaFe4Sb12 by three-axis inelastic neutron spectroscopy. The dispersion of phonons with wave vectors q along [ xx 0 ] and [ xxx ] directions in the energy range of eigenmodes with high amplitudes of lanthanum vibrations, i.e., at ℏω < 12 meV is identified. Symmetry-avoided anticrossing dispersion of phonons is established in both monitored directions and distinct eigenstates at high-symmetry points and at the Brillouin-zone center are discriminated. The experimentally derived phonon dispersion and intensities are compared with and backed up by ab initio lattice dynamics calculations. results of the computer model match well with the experimental data.

  5. Poly(3-methylpyrrole): vibrational dynamics, phonon dispersion and heat capacity.

    PubMed

    Ali, Parvej; Srivastava, Seema; Ansari, Saif-ul-Islam; Gupta, V D

    2013-07-01

    Normal modes of vibration and their dispersions in poly(3-methylpyrrole) (P3MPy) based on the Urey-Bradley force field are reported. It provides a detailed interpretation of previously reported I.R. spectra. Characteristic features of dispersion curves, such as regions of high density-of-states, repulsion, and character mixing of dispersive modes are discussed. Predictive values of heat capacity as a function of temperature are calculated from dispersion curves via density-of-states.

  6. Poly(3-methylpyrrole): Vibrational dynamics, phonon dispersion and heat capacity

    NASA Astrophysics Data System (ADS)

    Ali, Parvej; Srivastava, Seema; Ansari, Saif-ul-Islam; Gupta, V. D.

    2013-07-01

    Normal modes of vibration and their dispersions in poly(3-methylpyrrole) (P3MPy) based on the Urey-Bradley force field are reported. It provides a detailed interpretation of previously reported I.R. spectra. Characteristic features of dispersion curves, such as regions of high density-of-states, repulsion, and character mixing of dispersive modes are discussed. Predictive values of heat capacity as a function of temperature are calculated from dispersion curves via density-of-states.

  7. Decoupling of multiple coupled phononic crystal waveguides: application to acoustic demultiplexing

    NASA Astrophysics Data System (ADS)

    Zou, Qiushun; Liu, Wenxing; Yu, Tianbao; Liu, Nianhua; Wang, Tongbiao; Liao, Qinghua

    2017-03-01

    We show that the decoupling of two coupled phononic crystal waveguides (PnCWs) by a proper design can be achieved. And this decoupling property can be extended to the coupling of any number of parallel coupled PnCWs. The acoustic wavelength for decoupling is insensitive to the number of coupled PnCWs. Decoupling induces the extinction of neighbor PnCWs’ power transfer and makes the design of compact acoustic components easier. As a possible application of our work, a new kind of 1-to-2 acoustic demultiplexers are numerically demonstrated by employing the decoupling at the crossing-point frequency in two and three coupled PnCWs. This design concept provides a novel method and compact model for acoustic demultiplexing and can present practical applications in future acoustic wave circuits.

  8. Dispersion of Phonon Surface Polaritons in ZnGeP2: Anisotropy and Temperature Impacts

    NASA Astrophysics Data System (ADS)

    Shportko, K. V.; Otto, A.; Venger, E. F.

    2016-02-01

    Zinc germanium diphosphide (ZnGeP2) is an attractive and promising functional material for different devices of the nano- and optoelectronics. In this paper, dispersion of phonon surface polaritons (PSPs) in ZnGeP2 has been studied in the 200-500-cm-1 spectral range at 4 and 300 K. Dispersion of "real" and "virtual" PSPs were calculated for C-axis being normal and parallel to the surface. Anisotropy in ZnGeP2 leads to the different numbers of PSP dispersion branches for different orientations of the sample. The temperature-dependent phonon contributions in the dielectric permittivity shift dispersion of the surface polaritons in ZnGeP2 to the higher wavenumbers at 4 K. We have shown that experimental dispersion of PSP is in agreement with theory.

  9. Real-time observation of coherent acoustic phonons generated by an acoustically mismatched optoacoustic transducer using x-ray diffraction

    SciTech Connect

    Persson, A. I. H.; Andreasson, B. P.; Enquist, H.; Jurgilaitis, A.; Larsson, J.

    2015-11-14

    The spectrum of laser-generated acoustic phonons in indium antimonide coated with a thin nickel film has been studied using time-resolved x-ray diffraction. Strain pulses that can be considered to be built up from coherent phonons were generated in the nickel film by absorption of short laser pulses. Acoustic reflections at the Ni–InSb interface leads to interference that strongly modifies the resulting phonon spectrum. The study was performed with high momentum transfer resolution together with high time resolution. This was achieved by using a third-generation synchrotron radiation source that provided a high-brightness beam and an ultrafast x-ray streak camera to obtain a temporal resolution of 10 ps. We also carried out simulations, using commercial finite element software packages and on-line dynamic diffraction tools. Using these tools, it is possible to calculate the time-resolved x-ray reflectivity from these complicated strain shapes. The acoustic pulses have a peak strain amplitude close to 1%, and we investigated the possibility to use this device as an x-ray switch. At a bright source optimized for hard x-ray generation, the low reflectivity may be an acceptable trade-off to obtain a pulse duration that is more than an order of magnitude shorter.

  10. Long-Lived, Coherent Acoustic Phonon Oscillations in GaN Single Crystals

    SciTech Connect

    Wu, S.; Geiser, P.; Jun, J.; Karpinski, J.; Park, J.-R.; Sobolewski, R.

    2006-01-31

    We report on coherent acoustic phonon (CAP) oscillations studied in high-quality bulk GaN single crystals with a two-color femtosecond optical pump-probe technique. Using a far-above-the-band gap ultraviolet excitation (~270 nm wavelength) and a near-infrared probe beam (~810 nm wavelength), the long-lived, CAP transients were observed within a 10 ns time-delay window between the pump and probe pulses, with a dispersionless (proportional to the probe-beam wave vector) frequency of ~45 GHz. The measured CAP attenuation corresponded directly to the absorption of the probe light in bulk GaN, indicating that the actual (intrinsic) phonon-wave attenuation in our crystals was significantly smaller than the measured 65.8 cm^-1 value. The velocity of the phonon propagation was equal to the velocity of sound in GaN.

  11. Piezoelectric Response to Coherent Longitudinal and Transverse Acoustic Phonons in a Semiconductor Schottky Diode

    NASA Astrophysics Data System (ADS)

    Srikanthreddy, D.; Glavin, B. A.; Poyser, C. L.; Henini, M.; Lehmann, D.; Jasiukiewicz, Cz.; Akimov, A. V.; Kent, A. J.

    2017-02-01

    We study the generation of microwave electronic signals by pumping a (311) GaAs Schottky diode with compressive and shear acoustic phonons, generated by the femtosecond optical excitation of an Al film transducer and mode conversion at the Al-GaAs interface. They propagate through the substrate and arrive at the Schottky device on the opposite surface, where they induce a microwave electronic signal. The arrival time, the amplitude, and the polarity of the signals depend on the phonon mode. A theoretical analysis is made of the polarity of the experimental signals. This analysis includes the piezoelectric and deformation potential mechanisms of electron-phonon interaction in a Schottky contact and shows that the piezoelectric mechanism is dominant for both transverse and longitudinal modes with frequencies below 250 and 70 GHz, respectively.

  12. Acoustic beam splitting in two-dimensional phononic crystals using self-collimation effect

    SciTech Connect

    Li, Jing; Wu, Fugen Zhong, Huilin; Yao, Yuanwei; Zhang, Xin

    2015-10-14

    We propose two models of self-collimation-based beam splitters in phononic crystals. The finite element method is used to investigate the propagation properties of acoustic waves in two-dimensional phononic crystals. The calculated results show that the efficiency of the beam splitter can be controlled systematically by varying the radius of the rods or by changing the orientation of the square rods in the line defect. The effect of changing the side length of the square rods on acoustic wave propagation is discussed. The results show that the total transmission/reflection range decreases/increases as the side length increases. We also find that the relationship between the orientation of the transflective point and the side length of the square rods is quasi-linear.

  13. Cooling phonons with phonons: Acoustic reservoir engineering with silicon-vacancy centers in diamond

    NASA Astrophysics Data System (ADS)

    Kepesidis, K. V.; Lemonde, M.-A.; Norambuena, A.; Maze, J. R.; Rabl, P.

    2016-12-01

    We study a setup where a single negatively-charged silicon-vacancy center in diamond is magnetically coupled to a low-frequency mechanical bending mode and via strain to the high-frequency phonon continuum of a semiclamped diamond beam. We show that under appropriate microwave driving conditions, this setup can be used to induce a laser-cooling-like effect for the low-frequency mechanical vibrations, where the high-frequency longitudinal compression modes of the beam serve as an intrinsic low-temperature reservoir. We evaluate the experimental conditions under which cooling close to the quantum ground state can be achieved and describe an extended scheme for the preparation of a stationary entangled state between two mechanical modes. By relying on intrinsic properties of the mechanical beam only, this approach offers an interesting alternative for quantum manipulation schemes of mechanical systems, where otherwise efficient optomechanical interactions are not available.

  14. Demonstration of acoustic waveguiding and tight bending in phononic crystals

    DOE PAGES

    Ghasemi Baboly, M.; Raza, A.; Brady, J.; ...

    2016-10-31

    The systematic design, fabrication, and characterization of an isolated, single-mode, 90° bend phononic crystal (PnC) waveguide are presented. A PnC consisting of a 2D square array of circular air holes in an aluminum substrate is used, and waveguides are created by introducing a line defect in the PnC lattice. A high transmission coefficient is observed (–1 dB) for the straight sections of the waveguide, and an overall 2.3 dB transmission loss is observed (a transmission coefficient of 76%) for the 90° bend. Further optimization of the structure may yield higher transmission efficiencies. Lastly, this manuscript shows the complete design processmore » for an engineered 90° bend PnC waveguide from inception to experimental demonstration.« less

  15. Demonstration of acoustic waveguiding and tight bending in phononic crystals

    SciTech Connect

    Ghasemi Baboly, M.; Raza, A.; Brady, J.; Reinke, C. M.; Leseman, Z. C.; El-Kady, I.

    2016-10-31

    The systematic design, fabrication, and characterization of an isolated, single-mode, 90° bend phononic crystal (PnC) waveguide are presented. A PnC consisting of a 2D square array of circular air holes in an aluminum substrate is used, and waveguides are created by introducing a line defect in the PnC lattice. A high transmission coefficient is observed (–1 dB) for the straight sections of the waveguide, and an overall 2.3 dB transmission loss is observed (a transmission coefficient of 76%) for the 90° bend. Further optimization of the structure may yield higher transmission efficiencies. Lastly, this manuscript shows the complete design process for an engineered 90° bend PnC waveguide from inception to experimental demonstration.

  16. Anomalous negative reflection of acoustic waves from a two-dimensional phononic crystal immersed in water

    NASA Astrophysics Data System (ADS)

    Kang, Hwi Suk; Yoon, Suk Wang; Lee, Kang Il

    2017-02-01

    In the present study, we experimentally and theoretically demonstrated anomalous negative reflection of acoustic waves obliquely incident upon the boundary of a two-dimensional phononic crystal (PC) consisting of periodic square arrays of stainless-steel cylinders immersed in water. The angular spectrogram showing the frequency as a function of the angle was measured for the reflection from the PC when the incidence angle of the sound beam was fixed to be 20°. To understand the negative reflection from the PC, we considered the boundary of the PC to behave as an acoustic diffraction grating, and we calculated the acoustic pressure fields at specific frequencies of interest by using the finite element method. We found that the grating law could be successfully applied to the boundary of the PC in order to determine the direction of the acoustic waves diffracted in water.

  17. Effective field theory and dispersion law of the phonons of a nonrelativistic superfluid

    SciTech Connect

    Escobedo, Miguel Angel; Manuel, Cristina

    2010-08-15

    We study the recently proposed effective-field theory for the phonon of an arbitrary nonrelativistic superfluid. After computing the one-loop phonon self-energy, we obtain the low-temperature T contributions to the phonon dispersion law at low momentum and see that the real part of those can be parametrized as a thermal correction to the phonon velocity. Because the phonons are the quanta of the sound waves, at low momentum their velocity should agree with the speed of sound. We find that our results match at order T{sup 4}lnT with those predicted by Andreev and Khalatnikov for the speed of sound, derived from the superfluid hydrodynamical equations and the phonon kinetic theory. We get also higher-order corrections of order T{sup 4}, which are not reproduced pushing naively the kinetic theory computation. Finally, as an application, we consider the cold Fermi gas in the unitarity limit and find a universal expression for the low-T relative correction to the speed of sound for these systems.

  18. Anisotropic surface phonon dispersion of the hydrogen-terminated Si(110)-(1×1) surface: One-dimensional phonons propagating along the glide planes

    SciTech Connect

    Matsushita, Stephane Yu; Matsui, Kazuki; Kato, Hiroki; Suto, Shozo; Yamada, Taro

    2014-03-14

    We have measured the surface phonon dispersion curves on the hydrogen-terminated Si(110)-(1×1) surface with the two-dimensional space group of p2mg along the two highly symmetric and rectangular directions of ΓX{sup ¯} and ΓX{sup ′¯} using high-resolution electron-energy-loss spectroscopy. All the essential energy-loss peaks on H:Si(110) were assigned to the vibrational phonon modes by using the selection rules of inelastic electron scattering including the glide-plane symmetry. Actually, the surface phonon modes of even-symmetry to the glide plane (along ΓX{sup ¯}) were observed in the first Brillouin zone, and those of odd-symmetry to the glide plane were in the second Brillouin zone. The detailed assignment was made by referring to theoretical phonon dispersion curves of Gräschus et al. [Phys. Rev. B 56, 6482 (1997)]. We found that the H–Si stretching and bending modes, which exhibit highly anisotropic dispersion, propagate along ΓX{sup ¯} direction as a one-dimensional phonon. Judging from the surface structure as well as our classical and quantum mechanical estimations, the H–Si stretching phonon propagates by a direct repulsive interaction between the nearest neighbor H atoms facing each other along ΓX{sup ¯}, whereas the H–Si bending phonon propagates by indirect interaction through the substrate Si atomic linkage.

  19. Intrinsic coherent acoustic phonons in the indirect band gap semiconductors Si and GaP

    NASA Astrophysics Data System (ADS)

    Ishioka, Kunie; Rustagi, Avinash; Höfer, Ulrich; Petek, Hrvoje; Stanton, Christopher J.

    2017-01-01

    We report on the intrinsic optical generation and detection of coherent acoustic phonons at (001)-oriented bulk Si and GaP without metallic phonon transducer structures. Photoexcitation by a 3.1-eV laser pulse generates a normal strain pulse within the ˜100 -nm penetration depth in both semiconductors. The subsequent propagation of the strain pulse into the bulk is detected with a delayed optical probe as a periodic modulation of the optical reflectivity. Our theoretical model explains quantitatively the generation of the acoustic pulse via the deformation potential electron-phonon coupling and detection in terms of the spatially and temporally dependent photoelastic effect for both semiconductors. Comparison with our theoretical model reveals that the experimental strain pulses have finite buildup times of 1.2 and 0.4 ps for GaP and Si, which are comparable with the time required for the photoexcited electrons to transfer to the lowest X valley through intervalley scattering. The deformation potential coupling related to the acoustic pulse generation for GaP is estimated to be twice as strong as that for Si from our experiments, in agreement with a previous theoretical prediction.

  20. Finite element analysis of true and pseudo surface acoustic waves in one-dimensional phononic crystals

    SciTech Connect

    Graczykowski, B. Alzina, F.; Gomis-Bresco, J.; Sotomayor Torres, C. M.

    2016-01-14

    In this paper, we report a theoretical investigation of surface acoustic waves propagating in one-dimensional phononic crystal. Using finite element method eigenfrequency and frequency response studies, we develop two model geometries suitable to distinguish true and pseudo (or leaky) surface acoustic waves and determine their propagation through finite size phononic crystals, respectively. The novelty of the first model comes from the application of a surface-like criterion and, additionally, functional damping domain. Exemplary calculated band diagrams show sorted branches of true and pseudo surface acoustic waves and their quantified surface confinement. The second model gives a complementary study of transmission, reflection, and surface-to-bulk losses of Rayleigh surface waves in the case of a phononic crystal with a finite number of periods. Here, we demonstrate that a non-zero transmission within non-radiative band gaps can be carried via leaky modes originating from the coupling of local resonances with propagating waves in the substrate. Finally, we show that the transmission, reflection, and surface-to-bulk losses can be effectively optimised by tuning the geometrical properties of a stripe.

  1. Observing backfolded and unfolded acoustic phonons by broadband optical light scattering.

    PubMed

    Maerten, L; Bojahr, A; Bargheer, M

    2015-02-01

    We use broadband time domain Brillouin scattering to observe coherently generated phonon modes in bulk and nanolayered samples. We transform the measured transients into a frequency-wavevector diagram and compare the resulting dispersion relations to calculations. The detected oscillation amplitude depends on the occupation of phonon modes induced by the pump pulse. For nanolayered samples with an appropriately large period, the whole wavevector range of the Brillouin zone becomes observable by broadband optical light scattering. The backfolded modes vanish, when the excitation has passed the nanolayers and propagates through the substrate underneath.

  2. Understanding Vibrational Anharmonicity and Phonon Dispersion in Solid Ammonia Borane

    SciTech Connect

    Kathmann, Shawn M.; Mundy, Christopher J.; Schenter, Gregory K.; Autrey, Thomas; Aeberhard, Philippe C.; David, William; Jones, Martin O.; Ramirez-Cuesta, Timmy

    2012-03-08

    We compute the hydrogen vibrational spectra for bulk ammonia borane (NH3BH3) using harmonic and anharmonic methodologies as well as quantifying dispersive effects to determine their influence on the resulting spectra. Even at 10K the accounting of anharmonic effects on the IINS signal are more significant than approximations introduced by sampling and interpolating a finite simulation cell to capture dispersion effects. We compare our computed anharmonic power spectrum with IINS spectral measurements and find excellent agreement. This work was supported by the US Department of Energy Basic Energy Sciences' Chemical Sciences, Geosciences and Biosciences Division. Pacific Northwest National Laboratory is operated by Battelle for the US Department of Energy.

  3. Ultra-wide acoustic band gaps in pillar-based phononic crystal strips

    NASA Astrophysics Data System (ADS)

    Coffy, Etienne; Lavergne, Thomas; Addouche, Mahmoud; Euphrasie, Sébastien; Vairac, Pascal; Khelif, Abdelkrim

    2015-12-01

    An original approach for designing a one dimensional phononic crystal strip with an ultra-wide band gap is presented. The strip consists of periodic pillars erected on a tailored beam, enabling the generation of a band gap that is due to both Bragg scattering and local resonances. The optimized combination of both effects results in the lowering and the widening of the main band gap, ultimately leading to a gap-to-midgap ratio of 138%. The design method used to improve the band gap width is based on the flattening of phononic bands and relies on the study of the modal energy distribution within the unit cell. The computed transmission through a finite number of periods corroborates the dispersion diagram. The strong attenuation, in excess of 150 dB for only five periods, highlights the interest of such ultra-wide band gap phononic crystal strips.

  4. Ultra-wide acoustic band gaps in pillar-based phononic crystal strips

    SciTech Connect

    Coffy, Etienne Lavergne, Thomas; Addouche, Mahmoud; Euphrasie, Sébastien; Vairac, Pascal; Khelif, Abdelkrim

    2015-12-07

    An original approach for designing a one dimensional phononic crystal strip with an ultra-wide band gap is presented. The strip consists of periodic pillars erected on a tailored beam, enabling the generation of a band gap that is due to both Bragg scattering and local resonances. The optimized combination of both effects results in the lowering and the widening of the main band gap, ultimately leading to a gap-to-midgap ratio of 138%. The design method used to improve the band gap width is based on the flattening of phononic bands and relies on the study of the modal energy distribution within the unit cell. The computed transmission through a finite number of periods corroborates the dispersion diagram. The strong attenuation, in excess of 150 dB for only five periods, highlights the interest of such ultra-wide band gap phononic crystal strips.

  5. Wave propagation and acoustic band gaps of two-dimensional liquid crystal/solid phononic crystals

    NASA Astrophysics Data System (ADS)

    Oltulu, Oral; Mamedov, Amirullah M.; Ozbay, Ekmel

    2017-01-01

    The vast majority of acoustic wave propagation in phononic band studies has been usually carried out by scattering inclusions embedded in a viscoelastic medium, such as air or water. In this study, we present calculated band structure results for the two-dimensional square array geometry of a solid cylindrical scatterer surrounded by a liquid crystal (LC) matrix. Liquid crystals provide a unique combination of liquid-like and crystal-like properties as well as anisotropic properties. The purpose of using LC material is to take advantage of longitudinal acoustic waves propagating parallel (||) and perpendicular (⊥) to the nematic liquid crystal (NLC) director n. The compound used in this study was a room temperature NLC, called 5CB (4-pentyl-4'-cyanobiphenyl). The acoustic band structure of a two-dimensional phononic crystal containing a 5CB NLC and lithium tantalate was investigated by the plane wave expansion method. The theoretical results show that the solid/LC system can be tuned in a favorable configuration for adjusting or shifting acoustic band gaps.

  6. A first principle study for the comparison of phonon dispersion of armchair carbon and silicon nanotubes

    SciTech Connect

    Chandel, Surjeet Kumar; Kumar, Arun; Bharti, Ankush; Sharma, Raman

    2015-05-15

    Using first principles density functional theoretical calculations, the present paper reports a systematic study of phonon dispersion curves in pristine carbon (CNT) and silicon nanotubes (SiNT) having chirality (6,6) in the armchair configuration. Some of the phonon modes are found to have negative frequencies which leads to instability of the systems under study. The number of phonon branches has been found to be thrice as much as the number of atoms. The frequency of the higher optical bands varies from 1690 to 1957 cm{sup −1} for CNT(6,6) while it is 596 to 658 cm{sup −1} for SiNT.

  7. Guiding and confinement of interface acoustic waves in solid-fluid pillar-based phononic crystals

    NASA Astrophysics Data System (ADS)

    Razip Wee, M. F. Mohd; Addouche, Mahmoud; Siow, Kim S.; Zain, A. R. Md; Elayouch, Aliyasin; Chollet, Franck; Khelif, Abdelkrim

    2016-12-01

    Pillar-based phononic crystals exhibit some unique wave phenomena due to the interaction between surface acoustic modes of the substrate and local resonances supported by pillars. In this paper, we extend the investigations by taking into account the presence of a liquid medium. We particularly demonstrate that local resonances dramatically decrease the phase velocity of Scholte-Stoneley wave, which leads to a slow wave at the solid/fluid interface. Moreover, we show that increasing the height of pillars introduces a new set of branches of interface modes and drastically affects the acoustic energy localization. Indeed, while some modes display a highly confined pressure between pillars, others exponentially decay in the fluid or only propagate in the solid without disturbing the fluid pressure. These theoretical results, performed by finite element method, highlight a new acoustic wave confinement suitable in various applications such as acoustophoresis, lab on chip and microfluidics.

  8. Probing Thermomechanics at the Nanoscale: Impulsively Excited Pseudosurface Acoustic Waves in Hypersonic Phononic Crystals

    PubMed Central

    2011-01-01

    High-frequency surface acoustic waves can be generated by ultrafast laser excitation of nanoscale patterned surfaces. Here we study this phenomenon in the hypersonic frequency limit. By modeling the thermomechanics from first-principles, we calculate the system’s initial heat-driven impulsive response and follow its time evolution. A scheme is introduced to quantitatively access frequencies and lifetimes of the composite system’s excited eigenmodes. A spectral decomposition of the calculated response on the eigemodes of the system reveals asymmetric resonances that result from the coupling between surface and bulk acoustic modes. This finding allows evaluation of impulsively excited pseudosurface acoustic wave frequencies and lifetimes and expands our understanding of the scattering of surface waves in mesoscale metamaterials. The model is successfully benchmarked against time-resolved optical diffraction measurements performed on one-dimensional and two-dimensional surface phononic crystals, probed using light at extreme ultraviolet and near-infrared wavelengths. PMID:21910426

  9. Dispersion and the electron-phonon interaction in a single heterostructure

    NASA Astrophysics Data System (ADS)

    Naylor, D. R.; Dyson, A.; Ridley, B. K.

    2017-02-01

    We investigate the electron-phonon interaction in a polar-polar single heterostructure through the use of the linear combination of hybrid phonon modes, considering the role of longitudinal optical, transverse optical and interface modes, using a continuum model that accounts for both mechanical and electrical continuity over a heterostructure interface. We discuss the use of other models for such systems, such as the bulk phonon (3DP) and dielectric continuum (DC) models, using previously developed sum-rules to explain the limitations on their validity. We find that our linear combination (LC) model gives an excellent agreement with scattering rates previously derived using the 3DP and DC models when the lattice dispersion is weak enough to be ignored, however, when there is a noticeable lattice dispersion, the LC model returns a different answer, suggesting that interface modes play a much greater part in the scattering characteristics of the system under certain conditions. We also discuss the remote phonon effect in polar/polar heterostructures.

  10. Phonon dispersion in austenitic stainless steel Fe18Cr12Ni2Mo

    NASA Astrophysics Data System (ADS)

    Hoelzel, M.; Danilkin, S. A.; Hoser, A.; Ehrenberg, H.; Wieder, T.; Fuess, H.

    The phonon dispersion of Fe18Cr12Ni2Mo austenitic stainless steel was measured along the symmetry directions [001], [110] and [111]. Data were analysed in the frame of the Born-von Karman model of lattice dynamics. The obtained force constants were used to evaluate the elastic constants and the engineering elastic moduli. Our results for the elastic constants confirm empirical relationships between the elastic constants found for FCC FeCrNi alloys.

  11. Coherent longitudinal acoustic phonons in three-dimensional supracrystals of cobalt nanocrystals.

    PubMed

    Lisiecki, Isabelle; Polli, Dario; Yan, Cong; Soavi, Giancarlo; Duval, Eugène; Cerullo, Giulio; Pileni, Marie-Paule

    2013-10-09

    We use broadband picosecond acoustics to detect longitudinal acoustic phonons with few-gigahertz frequency in three-dimensional supracrystals (with face-centered cubic lattice) of 7 nm cobalt nanocrystal spheres. In full analogy with atomic crystals, where longitudinal acoustic phonons propagate with the speed of sound through coherent movements of atoms of the lattice out of their equilibrium positions, in these supracrystals atoms are replaced by (uncompressible) nanocrystals and atomic bonds by coating agents (carbon chains) that act like mechanical springs holding together the nanocrystals. By repeating the measurements at different laser angles of incidence it was possible to accurately determine both the index of refraction of the supracrystal (n = 1.26 ± 0.03) and the room-temperature longitudinal speed of sound (v(s)= 1235 ± 12 m/s), which is quite low due to the heavy weight of the spheres (with respect to atoms in a crystal) and the soft carbon chains (with respect to atomic bonds). Interestingly, the speed of sound inside the supracrystal was found to dramatically increase by decreasing the sample temperature due to a change in the stiffness of the dodecanoic acid chains which coat the Co nanocrystals.

  12. Electron - polar acoustical phonon interactions in nitride based diluted magnetic semiconductor quantum well via hot electron magnetotransport

    SciTech Connect

    Pandya, Ankur; Shinde, Satyam; Jha, Prafulla K.

    2015-05-15

    In this paper the hot electron transport properties like carrier energy and momentum scattering rates and electron energy loss rates are calculated via interactions of electrons with polar acoustical phonons for Mn doped BN quantum well in BN nanosheets via piezoelectric scattering and deformation potential mechanisms at low temperatures with high electric field. Electron energy loss rate increases with the electric field. It is observed that at low temperatures and for low electric field the phonon absorption is taking place whereas, for sufficient large electric field, phonon emission takes place. Under the piezoelectric (polar acoustical phonon) scattering mechanism, the carrier scattering rate decreases with the reduction of electric field at low temperatures wherein, the scattering rate variation with electric field is limited by a specific temperature beyond which there is no any impact of electric field on such scattering.

  13. Controlled exciton transfer between quantum dots with acoustic phonons taken into account

    SciTech Connect

    Golovinski, P. A.

    2015-09-15

    A system of excitons in two quantum dots coupled by the dipole–dipole interaction is investigated. The excitation transfer process controlled by the optical Stark effect at nonresonant frequencies is considered and the effect of the interaction between excitons and acoustic phonons in a medium on this process is taken into account. The system evolution is described using quantum Heisenberg equations. A truncated set of equations is obtained and the transfer dynamics is numerically simulated. High-efficiency picosecond switching of the excitation transfer by a laser pulse with a rectangular envelope is demonstrated. The dependence of picosecond switching on the quantum-dot parameters and optical-pulse length is presented.

  14. Tunneling times of acoustic phonon packets through a distributed Bragg reflector

    PubMed Central

    2014-01-01

    The longwave phenomenological model is used to make simple and precise calculations of various physical quantities such as the vibrational energy density, the vibrational energy, the relative mechanical displacement, and the one-dimensional stress tensor of a porous silicon distributed Bragg reflector. From general principles such as invariance under time reversal, invariance under space reflection, and conservation of energy density flux, the equivalence of the tunneling times for both transmission and reflection is demonstrated. Here, we study the tunneling times of acoustic phonon packets through a distributed Bragg reflector in porous silicon multilayer structures, and we report the possibility that a phenomenon called Hartman effect appears in these structures. PMID:25237288

  15. Coherent acoustic phonon generation in GaAs{sub 1−x}Bi{sub x}

    SciTech Connect

    Joshya, R. S.; Kini, R. N.; Ptak, A. J.; France, R.; Mascarenhas, A.

    2014-03-03

    We have used femtosecond laser pulses to generate coherent acoustic phonons in the dilute Bismide alloy, GaAs{sub 1−x}Bi{sub x}. The observed oscillation periods match well with the oscillation periods calculated using the propagating strain pulse model. We attribute the generation process predominantly to electronic stress due to the absorption of the laser pulse at the surface of the GaAs{sub 1−x}Bi{sub x} layer. Our initial estimates suggest that the incorporation of Bi in GaAs causes an enhancement of the hydrostatic deformation potential because of the resonant state in the valence band due to isolated Bi impurities.

  16. Shear-horizontal surface acoustic wave phononic device with high density filling material for ultra-low power sensing applications

    SciTech Connect

    Richardson, M.; Bhethanabotla, V. R.; Sankaranarayanan, S. K. R. S.

    2014-06-23

    Finite element simulations of a phononic shear-horizontal surface acoustic wave (SAW) sensor based on ST 90°-X Quartz reveal a dramatic reduction in power consumption. The phononic sensor is realized by artificially structuring the delay path to form an acoustic meta-material comprised of a periodic microcavity array incorporating high-density materials such as tantalum or tungsten. Constructive interference of the scattered and secondary reflected waves at every microcavity interface leads to acoustic energy confinement in the high-density regions translating into reduced power loss. Tantalum filled cavities show the best performance while tungsten inclusions create a phononic bandgap. Based on our simulation results, SAW devices with tantalum filled microcavities were fabricated and shown to significantly decrease insertion loss. Our findings offer encouraging prospects for designing low power, highly sensitive portable biosensors.

  17. Continuum approach for long-wavelength acoustic phonons in quasi-two-dimensional structures

    NASA Astrophysics Data System (ADS)

    Liu, Dan; Every, Arthur G.; Tománek, David

    2016-10-01

    As an alternative to atomistic calculations of long-wavelength acoustic modes of atomically thin layers, which are known to converge very slowly, we propose a quantitatively predictive and physically intuitive approach based on continuum elasticity theory. We describe a layer, independent of its thickness, by a membrane and characterize its elastic behavior by a (3 ×3 ) elastic matrix as well as the flexural rigidity. We present simple quantitative expressions for frequencies of long-wavelength acoustic modes, which we determine using two-dimensional elastic constants calculated by ab initio density functional theory. The calculated spectra accurately reproduce observed and calculated long-wavelength phonon spectra of graphene and phosphorene, the monolayer of black phosphorus. Our approach also correctly describes the observed dependence of the radial breathing mode frequency on the diameters of carbon fullerenes and nanotubes.

  18. Amplification of terahertz frequency acoustic phonons by drifting electrons in three-dimensional Dirac semimetals

    NASA Astrophysics Data System (ADS)

    Bhargavi, K. S.; Kubakaddi, S. S.

    2016-09-01

    The amplification coefficient α of acoustic phonons is theoretically investigated in a three-dimensional Dirac semimetal (3DDS) driven by a dc electric field E causing the drift of the electrons. It is numerically studied as a function of the frequency ωq, drift velocity vd, electron concentration ne, and temperature T in the Dirac semimetal Cd3As2. We find that the amplification of acoustic phonons (α ˜ hundreds of cm-1) takes place when the electron drift velocity vd is greater than the sound velocity vs. The amplification is found to occur at small E (˜few V/cm) due to large electron mobility. The frequency dependence of α shows amplification in the THz regime with a maximum αm occurring at the same frequency ωqm for different vd. The αm is found to increase with increasing vd. α vs ωq for different ne also shows a maximum, with αm shifting to higher ωq for larger ne. Each maximum is followed by a vanishing α at nearly "2kf cutoff," where kf is the Fermi wave vector. It is found that αm/ne and ωqm/ne1/3 are nearly constant. The αm ˜ ne can be used to identify the 3DDS phase as it differs from αm ˜ ne1/3 dependence in conventional bulk Cd3As2 semiconductor.

  19. Compositional Variation of the Phonon Dispersion Curves of bcc Fe-Ga Alloys

    SciTech Connect

    Zarestky, Jerel L; Garlea, Vasile O; Lograsso, Tom; Schlagel, D. L.; Stassis, C.

    2005-01-01

    Inelastic neutron scattering techniques have been used to measure the phonon dispersion curves of bcc Fe1?xGax x=10.8, 13.3, 16.0, 22.5 alloys as a function of Ga concentration. The phonon frequencies of every branch were found to decrease significantly with increasing Ga concentration. The softening was most pronounced for the T2 0 branch and, to a lesser extent, the L branch in the vicinity of = 2 3. The concentration dependence of the shear elastic constant C =1/2 C11?C12 , calculated from the slope of the T2 0 branch, was found to agree with the results of sound velocity measurements. For the higher concentration sample measured, 22.5 at. % Ga, new branches appeared, an effect associated with the increase in the number of atoms per unit cell.

  20. Particle filtering for dispersion curve tracking in ocean acoustics.

    PubMed

    Zorych, Ivan; Michalopoulou, Zoi-Heleni

    2008-08-01

    A particle filtering method is developed for dispersion curve extraction from spectrograms of broadband acoustic signals propagating in underwater media. The goal is to obtain accurate representation of modal dispersion which can be employed for source localization and geoacoustic inversion. Results are presented from the application of the method to synthetic data, demonstrating the potential of the approach for accurate estimation of waveguide dispersion characteristics. The method outperforms simple time-frequency analysis providing estimates that are very close to numerically calculated dispersion curves. The method also provides uncertainty information on modal arrival time estimates, typically unavailable when traditional methods are used.

  1. A structural mechanics approach for the phonon dispersion analysis of graphene

    NASA Astrophysics Data System (ADS)

    Hou, X. H.; Deng, Z. C.; Zhang, K.

    2017-04-01

    A molecular structural mechanics model for the numerical simulation of phonon dispersion relations of graphene is developed by relating the C-C bond molecular potential energy to the strain energy of the equivalent beam-truss space frame. With the stiffness matrix known and further based on the periodic structure characteristics, the Bloch theorem is introduced to develop the dispersion relation of graphene sheet. Being different from the existing structural mechanics model, interactions between the fourth-nearest neighbor atoms are further simulated with beam elements to compensate the reduced stretching stiffness, where as a result not only the dispersion relations in the low frequency field are accurately achieved, but results in the high frequency field are also reasonably obtained. This work is expected to provide new opportunities for the dynamic properties analysis of graphene and future application in the engineering sector.

  2. Phonon dispersion curves determination in (delta)-phase Pu-Ga alloys

    SciTech Connect

    Wong, J; Clatterbuck, D; Occelli, F; Farber, D; Schwartz, A; Wall, M; Boro, C; Krisch, M; Beraud, A; Chiang, T; Xu, R; Hong, H; Zschack, P; Tamura, N

    2006-02-07

    We have designed and successfully employed a novel microbeam on large grain sample concept to conduct high resolution inelastic x-ray scattering (HRIXS) experiments to map the full phonon dispersion curves of an fcc {delta}-phase Pu-Ga alloy. This approach obviates experimental difficulties with conventional inelastic neutron scattering due to the high absorption cross section of the common {sup 239}Pu isotope and the non-availability of large (mm size) single crystal materials for Pu and its alloys. A classical Born von-Karman force constant model was used to model the experimental results, and no less than 4th nearest neighbor interactions had to be included to account for the observation. Several unusual features including, a large elastic anisotropy, a small shear elastic modulus, (C{sub 11}-C{sub 12})/2, a Kohn-like anomaly in the T{sub 1}[011] branch, and a pronounced softening of the T[111] branch towards the L point in the Brillouin are found. These features may be related to the phase transitions of plutonium and to strong coupling between the crystal structure and the 5f valence instabilities. Our results represent the first full phonon dispersions ever obtained for any Pu-bearing material, thus ending a 40-year quest for this fundamental data. The phonon data also provide a critical test for theoretical treatments of highly correlated 5f electron systems as exemplified by recent dynamical mean field theory (DMFT) calculations for {delta}-plutonium. We also conducted thermal diffuse scattering experiments to study the T(111) dispersion at low temperatures with an attempt to gain insight into bending of the T(111) branch in relationship to the {delta} {yields} {alpha}{prime} transformation.

  3. Acoustic phonon dynamics in thin-films of the topological insulator Bi{sub 2}Se{sub 3}

    SciTech Connect

    Glinka, Yuri D.; Babakiray, Sercan; Johnson, Trent A.; Holcomb, Mikel B.; Lederman, David

    2015-04-28

    Transient reflectivity traces measured for nanometer-sized films (6–40 nm) of the topological insulator Bi{sub 2}Se{sub 3} revealed GHz-range oscillations driven within the relaxation of hot carriers photoexcited with ultrashort (∼100 fs) laser pulses of 1.51 eV photon energy. These oscillations have been suggested to result from acoustic phonon dynamics, including coherent longitudinal acoustic phonons in the form of standing acoustic waves. An increase of oscillation frequency from ∼35 to ∼70 GHz with decreasing film thickness from 40 to 15 nm was attributed to the interplay between two different regimes employing traveling-acoustic-waves for films thicker than 40 nm and the film bulk acoustic wave resonator (FBAWR) modes for films thinner than 40 nm. The amplitude of oscillations decays rapidly for films below 15 nm thick when the indirect intersurface coupling in Bi{sub 2}Se{sub 3} films switches the FBAWR regime to that of the Lamb wave excitation. The frequency range of coherent longitudinal acoustic phonons is in good agreement with elastic properties of Bi{sub 2}Se{sub 3}.

  4. Acoustic and electroacoustic spectroscopy for characterizing concentrated dispersions and emulsions.

    PubMed

    Dukhin, A S; Goetz, P J

    2001-09-03

    We describe two different techniques (acoustics and electroacoustics), both of which employ ultrasound instead of light for extracting information about the properties of liquid-based dispersions. Ultrasound can propagate through samples that are not transparent for light, which open up many new applications not possible with classical light scattering methods. Acoustic and electroacoustic techniques offer a unique opportunity to characterize concentrated dispersion, emulsions and microemulsions in their natural states. Elimination of a dilution step required for most other techniques (light scattering, sedimentation, electrophoresis) is crucial for an adequate characterization of liquid dispersions, especially when the high concentration leads to structured systems. As with any macroscopic method, ultrasonic techniques characterize the sample in two steps. The first step is to measure some macroscopic property. The second step involves some theoretical treatment of the measured raw data which yields the desired information. Acoustic spectroscopy deals with measuring the attenuation of ultrasound within a certain frequency range. Electroacoustic spectroscopy has two implementations depending on the driving force. We emphasize here on the so-called Colloid Vibration Current (CVI) which is generated by the sound wave as it passes through the dispersion. A review of the theoretical basis of acoustics and electroacoustics is given, with emphasis on models that have been applied to concentrated systems. Recently, new theories have been developed for both acoustics and electroacoustics using a 'coupled phase model' and 'cell model concept'. The coupled phase model is widely used for describing a relative motion of the particles and liquid in the sound wave. The cell model approach opens the way to include both particle-particle interactions and polydispersity into the theoretical model. Experimental evidence is presented that shows that this new approach is successful in

  5. Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites

    PubMed Central

    Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W.; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin

    2017-01-01

    The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA+/MA+/Cs+, X=I−/Br−) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials. PMID:28106061

  6. Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites.

    PubMed

    Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin

    2017-01-20

    The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA(+)/MA(+)/Cs(+), X=I(-)/Br(-)) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials.

  7. Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites

    NASA Astrophysics Data System (ADS)

    Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W.; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin

    2017-01-01

    The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA+/MA+/Cs+, X=I-/Br-) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials.

  8. Beam paths of flexural Lamb waves at high frequency in the first band within phononic crystal-based acoustic lenses

    SciTech Connect

    Zhao, J.; Boyko, O.; Bonello, B.

    2014-12-15

    This work deals with an analytical and numerical study of the focusing of the lowest order anti-symmetric Lamb wave in gradient index phononic crystals. Computing the ray trajectories of the elastic beam allowed us to analyze the lateral dimensions and shape of the focus, either in the inner or behind the phononic crystal-based acoustic lenses, for frequencies within a broad range in the first band. We analyzed and discussed the focusing behaviors inside the acoustic lenses where the focalization at sub-wavelength scale was achieved. The focalization behind the gradient index phononic crystal is shown to be efficient as well: we report on FMHM = 0.63λ at 11MHz.

  9. Lattice vibrations in the Frenkel-Kontorova model. I. Phonon dispersion, number density, and energy

    DOE PAGES

    Meng, Qingping; Wu, Lijun; Welch, David O.; ...

    2015-06-17

    We studied the lattice vibrations of two inter-penetrating atomic sublattices via the Frenkel-Kontorova (FK) model of a linear chain of harmonically interacting atoms subjected to an on-site potential, using the technique of thermodynamic Green's functions based on quantum field-theoretical methods. General expressions were deduced for the phonon frequency-wave-vector dispersion relations, number density, and energy of the FK model system. In addition, as the application of the theory, we investigated in detail cases of linear chains with various periods of the on-site potential of the FK model. Some unusual but interesting features for different amplitudes of the on-site potential of themore » FK model are discussed. In the commensurate structure, the phonon spectrum always starts at a finite frequency, and the gaps of the spectrum are true ones with a zero density of modes. In the incommensurate structure, the phonon spectrum starts from zero frequency, but at a non-zero wave vector; there are some modes inside these gap regions, but their density is very low. In our approximation, the energy of a higher-order commensurate state of the one-dimensional system at a finite temperature may become indefinitely close to the energy of an incommensurate state. This finding implies that the higher-order incommensurate-commensurate transitions are continuous ones and that the phase transition may exhibit a “devil's staircase” behavior at a finite temperature.« less

  10. Lattice vibrations in the Frenkel-Kontorova model. I. Phonon dispersion, number density, and energy

    SciTech Connect

    Meng, Qingping; Wu, Lijun; Welch, David O.; Zhu, Yimei

    2015-06-17

    We studied the lattice vibrations of two inter-penetrating atomic sublattices via the Frenkel-Kontorova (FK) model of a linear chain of harmonically interacting atoms subjected to an on-site potential, using the technique of thermodynamic Green's functions based on quantum field-theoretical methods. General expressions were deduced for the phonon frequency-wave-vector dispersion relations, number density, and energy of the FK model system. In addition, as the application of the theory, we investigated in detail cases of linear chains with various periods of the on-site potential of the FK model. Some unusual but interesting features for different amplitudes of the on-site potential of the FK model are discussed. In the commensurate structure, the phonon spectrum always starts at a finite frequency, and the gaps of the spectrum are true ones with a zero density of modes. In the incommensurate structure, the phonon spectrum starts from zero frequency, but at a non-zero wave vector; there are some modes inside these gap regions, but their density is very low. In our approximation, the energy of a higher-order commensurate state of the one-dimensional system at a finite temperature may become indefinitely close to the energy of an incommensurate state. This finding implies that the higher-order incommensurate-commensurate transitions are continuous ones and that the phase transition may exhibit a “devil's staircase” behavior at a finite temperature.

  11. Reflection thermal diffuse x-ray scattering for quantitative determination of phonon dispersion relations

    DOE PAGES

    Mei, A. B.; Hellman, O.; Schlepuetz, C. M.; ...

    2015-11-03

    Synchrotron reflection x-ray thermal diffuse scattering (TDS) measurements, rather than previously reported transmission TDS, are carried out at room temperature and analyzed using a formalism based upon second-order interatomic force constants and long-range Coulomb interactions to obtain quantitative determinations of MgO phonon dispersion relations (h) over bar omega(j) (q), phonon densities of states g((h) over bar omega), and isochoric temperature-dependent vibrational heat capacities cv (T). We use MgO as a model system for investigating reflection TDS due to its harmonic behavior as well as its mechanical and dynamic stability. Resulting phonon dispersion relations and densities of states are found tomore » be in good agreement with independent reports from inelastic neutron and x-ray scattering experiments. Temperature-dependent isochoric heat capacities cv (T), computed within the harmonic approximation from (h) over bar omega(j) (q) values, increase with temperature from 0.4 x 10-4 eV/atom K at 100 K to 1.4 x 10-4 eV/atom K at 200 K and 1.9 x 10-4 eV/atom K at 300 K, in excellent agreement with isobaric heat capacity values cp (T) between 4 and 300 K. We anticipate that the experimental approach developed here will be valuable for determining vibrational properties of heteroepitaxial thin films since the use of grazing-incidence (θ ≲ θc where θc is the density-dependent critical angle) allows selective tuning of x-ray penetration depths to ≲ 10 nm.« less

  12. Thermodynamics and phonon dispersion of pyrope and grossular silicate garnets from ab initio simulations

    NASA Astrophysics Data System (ADS)

    Baima, Jacopo; Ferrabone, Matteo; Orlando, Roberto; Erba, Alessandro; Dovesi, Roberto

    2016-02-01

    The phonon dispersion and thermodynamic properties of pyrope ({Mg}_3{Al}_2{Si}_3{O}_{12}) and grossular ({Ca}_3{Al}_2{Si}_3{O}_{12} ) have been computed by using an ab initio quantum mechanical approach, an all-electron variational Gaussian-type basis set and the B3LYP hybrid functional, as implemented in the Crystal program. Dispersion effects in the phonon bands have been simulated by using supercells of increasing size, containing 80, 160, 320, 640, 1280 and 2160 atoms, corresponding to 1, 2, 4, 8, 16 and 27 {k} points in the first Brillouin zone. Phonon band structures, density of states and corresponding inelastic neutron scattering spectra are reported. Full convergence of the various thermodynamic properties, in particular entropy ( S) and specific heat at constant volume (CV), with the number of {k} points is achieved with 27 {k} points. The very regular behavior of the S( T) and CV(T) curves as a function of the number of {k} points, determined by high numerical stability of the code, permits extrapolation to an infinite number of {k} points. The limiting value differs from the 27-{k} case by only 0.40 % at 100 K for S (the difference decreasing to 0.11 % at 1000 K) and by 0.29 % (0.05 % at 1000 K) for CV. The agreement with the experimental data is rather satisfactory. We also address the problem of the relative entropy of pyrope and grossular, a still debated question. Our lattice dynamical calculations correctly describe the larger entropy of pyrope than grossular by taking into account merely vibrational contributions and without invoking "static disorder" of the Mg ions in dodecahedral sites. However, as the computed entropy difference is found to be larger than the experimental one by a factor of 2-3, present calculations cannot exclude possible thermally induced structural changes, which could lead to further conformational contributions to the entropy.

  13. Reflection thermal diffuse x-ray scattering for quantitative determination of phonon dispersion relations

    NASA Astrophysics Data System (ADS)

    Mei, A. B.; Hellman, O.; Schlepütz, C. M.; Rockett, A.; Chiang, T.-C.; Hultman, L.; Petrov, I.; Greene, J. E.

    2015-11-01

    Synchrotron reflection x-ray thermal diffuse scattering (TDS) measurements, rather than previously reported transmission TDS, are carried out at room temperature and analyzed using a formalism based upon second-order interatomic force constants and long-range Coulomb interactions to obtain quantitative determinations of MgO phonon dispersion relations ℏ ωj (q), phonon densities of states g (ℏ ω ), and isochoric temperature-dependent vibrational heat capacities cv(T ) . We use MgO as a model system for investigating reflection TDS due to its harmonic behavior as well as its mechanical and dynamic stability. Resulting phonon dispersion relations and densities of states are found to be in good agreement with independent reports from inelastic neutron and x-ray scattering experiments. Temperature-dependent isochoric heat capacities cv(T ) , computed within the harmonic approximation from ℏ ωj (q) values, increase with temperature from 0.4 ×10-4eV /atom K at 100 K to 1.4 ×10-4eV /atom K at 200 K and 1.9 ×10-4eV /atom K at 300 K, in excellent agreement with isobaric heat capacity values cp(T ) between 4 and 300 K. We anticipate that the experimental approach developed here will be valuable for determining vibrational properties of heteroepitaxial thin films since the use of grazing-incidence (θ ≲θc , where θc is the density-dependent critical angle) allows selective tuning of x-ray penetration depths to ≲10 nm .

  14. Reflection thermal diffuse x-ray scattering for quantitative determination of phonon dispersion relations

    SciTech Connect

    Mei, A. B.; Hellman, O.; Schlepuetz, C. M.; Rockett, A.; Chiang, T. -C.; Hultman, L.; Petrov, I.; Greene, J. E.

    2015-11-03

    Synchrotron reflection x-ray thermal diffuse scattering (TDS) measurements, rather than previously reported transmission TDS, are carried out at room temperature and analyzed using a formalism based upon second-order interatomic force constants and long-range Coulomb interactions to obtain quantitative determinations of MgO phonon dispersion relations (h) over bar omega(j) (q), phonon densities of states g((h) over bar omega), and isochoric temperature-dependent vibrational heat capacities cv (T). We use MgO as a model system for investigating reflection TDS due to its harmonic behavior as well as its mechanical and dynamic stability. Resulting phonon dispersion relations and densities of states are found to be in good agreement with independent reports from inelastic neutron and x-ray scattering experiments. Temperature-dependent isochoric heat capacities cv (T), computed within the harmonic approximation from (h) over bar omega(j) (q) values, increase with temperature from 0.4 x 10-4 eV/atom K at 100 K to 1.4 x 10-4 eV/atom K at 200 K and 1.9 x 10-4 eV/atom K at 300 K, in excellent agreement with isobaric heat capacity values cp (T) between 4 and 300 K. We anticipate that the experimental approach developed here will be valuable for determining vibrational properties of heteroepitaxial thin films since the use of grazing-incidence (θ ≲ θc where θc is the density-dependent critical angle) allows selective tuning of x-ray penetration depths to ≲ 10 nm.

  15. Tunability of acoustic phonon transmission and thermal conductance in three dimensional quasi-periodically stubbed waveguides

    NASA Astrophysics Data System (ADS)

    Xie, Zhong-Xiang; Liu, Jing-Zhong; Yu, Xia; Wang, Hai-Bin; Deng, Yuan-Xiang; Li, Ke-Min; Zhang, Yong

    2015-03-01

    We investigate acoustic phonon transmission and thermal conductance in three dimensional (3D) quasi-periodically stubbed waveguides according to the Fibonacci sequence. Results show that the transmission coefficient exhibits the periodic oscillation upon varying the length of stub/waveguide at low frequency, and the period of such oscillation is tunably decreased with increasing the Fibonacci number N. Interestingly, there also exist some anti-resonant dips that gradually develop into wide stop-frequency gaps with increasing N. As the temperature goes up, a transition of the thermal conductance from the decrease to the increase occurs in these systems. When N is increased, the thermal conductance is approximately decreased with a linear trend. Moreover, the decreasing degree sensitively depends on the variation of temperature. A brief analysis of these results is given.

  16. Precise parallel optical spectrum analysis using the advanced two-phonon light scattering combined with the cross-disperser technique.

    PubMed

    Shcherbakov, A S; Arellanes, A O; Chavushyan, V

    2016-12-01

    We develop an advanced approach to the optical spectrometer with acousto-optical dynamic grating for the Guillermo Haro astrophysical observatory (Mexico). The progress consists of two principle novelties. First is the use of the acousto-optical nonlinearity of two-phonon light scattering in crystals with linear acoustic losses. This advanced regime of light scattering exhibits a recently revealed additional degree of freedom, which allows tuning of the frequency of elastic waves and admits the nonlinear apodization improving the dynamic range. The second novelty is the combination of the cross-disperser with acousto-optical processing. A similar pioneering step provides an opportunity to operate over all the visible range in a parallel regime with maximal achievable resolution. The observation window of the optical spectrometer in that observatory is ∼9  cm, so that the theoretical estimations of maximal performances for a low-loss LiNbO3 crystal for this optical aperture at λ=405  nm give spectral resolution of 0.0523 Å, resolving power of 77,400, and 57,500 spots. The illustrative proof-of-principle experiments with a 6 cm LiNbO3 crystal have been performed.

  17. Dispersion of electron-phonon resonances in one-layer graphene and its demonstration in micro-Raman scattering.

    PubMed

    Strelchuk, V V; Nikolenko, A S; Gubanov, V O; Biliy, M M; Bulavin, L A

    2012-11-01

    In the present work, we used Raman spectroscopy as sensitive tool for characterization of dispersion of electron-phonon resonances in one-layer graphene. We analyzed Stokes and anti-Stokes components of the Raman spectra to investigate the temperature dependence of the graphene G-band on the power of exciting radiation. Appearance and drastic intensity increase of zone-edge D-like modes caused by introduction of structural defects and/or deformations in the graphene layer were observed in the Raman spectra at high powers of excitation. We investigated phonon dispersion of one-layer graphene for iTO phonon branch at K point along K-M direction, which is involved in double-resonance Raman scattering. Raman dispersion slope of D-band is in good agreement with results of theoretical calculations based on the Green's functions approach based on the screened electron-electron interaction. Deviation of the experimental iTO phonon frequency from the linear dependence on excitation energy was observed at excitation E(exc) = 3.81 eV. Self-consistent classification of phonon states according to the symmetry for all dispersion branches of one-layer graphene was carried out.

  18. CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES Phonon States and Dispersive Spectra of Polar Optical Phonons in Quasi-One-Dimensional Nanowires of Wurtzite ZnO and Zinc-Blend MgO Semiconductors

    NASA Astrophysics Data System (ADS)

    Zhang, Li

    2011-01-01

    Within the framework of the macroscopic dielectric continuum model and Loudon's uniaxial crystal model, the phonon modes of a wurtzite/zinc-blende one-dimensional (1D) cylindrical nanowire (NW) are derived and studied. The analytical phonon states of phonon modes are given. It is found that there exist two types of polar phonon modes, i.e. interface optical (IO) phonon modes and the quasi-confined (QC) phonon modes existing in 1D wurtzite/zinc-blende NWs. Via the standard procedure of field quantization, the Fröhlich electron-phonon interaction Hamiltonians are obtained. Numerical calculations of dispersive behavior of these phonon modes on a wurtzite/zinc-blende ZnO/MgO NW are performed. The frequency ranges of the IO and QC phonon modes of the ZnO/MgO NWs are analyzed and discussed. It is found that the IO modes only exist in one frequency range, while QC modes may appear in three frequency ranges. The dispersive properties of the IO and QC modes on the free wave-number kz and the azimuthal quantum number m are discussed. The analytical Hamiltonians of electron-phonon interaction obtained here are quite useful for further investigating phonon influence on optoelectronics properties of wurtzite/zinc-blende 1D NW structures.

  19. Observation of acoustic-phonon-like mode driven by magnetic imbalance between neighboring Fe atoms in Fe1+yTe (y < 0 . 12)

    NASA Astrophysics Data System (ADS)

    Fobes, David; Zaliznyak, Igor; Xu, Zhijun; Gu, Genda; Tranquada, John M.; He, Xu-Gang; Ku, Wei; Garlea, Ovidiu

    2014-03-01

    We have studied the evolution with temperature of the low-energy inelastic spectra of Fe1+yTe (y < 0 . 12), a parent compound of the iron-chalcogenide superconductor family, revealing an acoustic mode at an unexpected position. Recently, we found evidence for the formation of a bond-order wave leading to ferro-orbital order in the monoclinic phase, in part due to the observation of an elastic structural peak at (100) in the low-temperature monoclinic phase [D. Fobes, et al., arXiv:1307.7162]. In the inelastic spectra we observe a sharp acoustic-phonon-like mode dispersing out of the (100) position in the monoclinic phase. Surprisingly, the mode survives in the tetragonal phase, despite the absence of a Bragg peak at (100); such a peak is forbidden by symmetry. LDA calculations suggest this mode could involve significant magnetic scattering. By assuming in-phase virtual displacement of the Fe atoms from their equilibrium position in a frozen phonon calculation, we have found a small but significant imbalance in the magnetic moments between the two Fe atoms within the unit cell, suggesting magnetic contribution to the mode. Work at BNL supported by Office of Basic Energy Sciences, US DOE, under Contract No. DE-AC02-98CH10886. Research conducted at ORNL Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US DOE.

  20. The Numerical Solution of Acoustic Propagation through Dispersive Moving Media

    DTIC Science & Technology

    2010-06-01

    domain version [3] of the Kramer- Kronig relationships (K-K), [6] he arrived at a general form for the operator. Szabo’s operator was originally...for longitudinal and shear wave propagation in viscoelastic media,” J. Acoust. Soc. Am. 107, 2437-2446, 2000. [6] R. D. L. Kronig , “On the theory...domain representation of the Kramers- Kronig dispersion relations,” J. Acoust. Soc. Am. 108, 2114-2119, 2000. [8] G. V. Norton and J. C. Novarini

  1. Development of an acoustic filter for parametric loudspeaker using phononic crystals.

    PubMed

    Ji, Peifeng; Hu, Wenlin; Yang, Jun

    2016-04-01

    The spurious signal generated as a result of nonlinearity at the receiving system affects the measurement of the difference-frequency sound in the parametric loudspeaker, especially in the nearfield or near the beam axis. In this paper, an acoustic filter is designed using phononic crystals and its theoretical simulations are carried out by quasi-one- and two-dimensional models with Comsol Multiphysics. According to the simulated transmission loss (TL), an acoustic filter is prototyped consisting of 5×7 aluminum alloy cylinders and its performance is verified experimentally. There is good agreement with the simulation result for TL. After applying our proposed filter in the axial measurement of the parametric loudspeaker, a clear frequency dependence from parametric array effect is detected, which exhibits a good match with the well-known theory described by the Gaussian-beam expansion technique. During the directivity measurement for the parametric loudspeaker, the proposed filter has also proved to be effective and is only needed for small angles.

  2. Electron Transport Parameters Study for Transition Metal-Doped Armchair Graphene Nanoribbon via Acoustical Phonon Interactions

    NASA Astrophysics Data System (ADS)

    Pandya, Ankur; Jha, Prafulla K.

    2017-04-01

    Electron transport parameters such as electron effective mass, Fermi velocity of an electron and electron mobility are calculated for transition metal [manganese (Mn), cobalt (Co)]-doped armchair graphene nanoribbon (aGNR) via polar acoustical phonon [piezoelectric (PZ)] scattering and acoustical deformation potential (ADP) scattering under a high electric field and different doping concentrations. Moreover, the effect of dopant site on these electron transport parameters is also investigated. It is observed that the electron effective mass is reduced significantly in doped aGNR in comparison to pure GNR. It is observed that the net electron mobility contributed by both ADP and PZ mechanisms for Mn-doped aGNR as well as Co-doped aGNR varies in similar fashion as semiconductors wherein the net electron mobility (ADP + PZ) for Mn-doped aGNR is greater than that for the Co-doped graphene nanoribbon. Moreover, it is found that there is no impact of variation in dopant site on the electron transport parameters considered in this study.

  3. Optical absorption in semiconductor quantum dots coupling to dispersive phonons of infinite modes

    NASA Astrophysics Data System (ADS)

    Ding, Zhiwen; Wang, Qin; Zheng, Hang

    2012-10-01

    Optical absorption spectrum of semiconductor quantum dot is investigated by means of an analytical approach based on the Green's function for different forms of coupling strength in an unified method by using the standard model with valence and conduction band levels coupled to dispersive quantum phonons of infinite modes. The analytical expression of the optical absorption coefficient in semiconductor quantum dots is obtained and by this expression the line shape and the peak position of the absorption spectrum are procured. The relation between the properties of absorption spectrum and the forms of coupling strength is clarified, which can be referenced for choosing the proper form of the coupling strength or spectral density to control the features of absorption spectrum of quantum dot. The coupling and confinement induced energy shift and intensity decrease in the absorption spectrum are determined precisely for a wide range of parameters. The results show that the activation energy of the optical absorption is reduced by the effect of exciton-phonon coupling and photons with lower frequencies could also be absorbed in absorption process. With increase of the coupling constant, the line shape of optical absorption spectrum broadens and the peak position moves to lower photon energy with a rapid decrease in intensity at the same time. Both the coupling induced red shift and the confinement induced blue shift conduce to decrease in the intensity of absorption spectrum. Furthermore, this method may have application potential to other confined quantum systems.

  4. Engineering dissipation with phononic spectral hole burning.

    PubMed

    Behunin, R O; Kharel, P; Renninger, W H; Rakich, P T

    2017-03-01

    Optomechanics, nano-electromechanics, and integrated photonics have brought about a renaissance in phononic device physics and technology. Central to this advance are devices and materials supporting ultra-long-lived photonic and phononic excitations that enable novel regimes of classical and quantum dynamics based on tailorable photon-phonon coupling. Silica-based devices have been at the forefront of such innovations for their ability to support optical excitations persisting for nearly 1 billion cycles, and for their low optical nonlinearity. While acoustic phonon modes can persist for a similar number of cycles in crystalline solids at cryogenic temperatures, it has not been possible to achieve such performance in silica, as silica becomes acoustically opaque at low temperatures. We demonstrate that these intrinsic forms of phonon dissipation are greatly reduced (by >90%) by nonlinear saturation using continuous drive fields of disparate frequencies. The result is a form of steady-state phononic spectral hole burning that produces a wideband transparency window with optically generated phonon fields of modest (nW) powers. We developed a simple model that explains both dissipative and dispersive changes produced by phononic saturation. Our studies, conducted in a microscale device, represent an important step towards engineerable phonon dynamics on demand and the use of glasses as low-loss phononic media.

  5. Engineering dissipation with phononic spectral hole burning

    NASA Astrophysics Data System (ADS)

    Behunin, R. O.; Kharel, P.; Renninger, W. H.; Rakich, P. T.

    2016-12-01

    Optomechanics, nano-electromechanics, and integrated photonics have brought about a renaissance in phononic device physics and technology. Central to this advance are devices and materials supporting ultra-long-lived photonic and phononic excitations that enable novel regimes of classical and quantum dynamics based on tailorable photon-phonon coupling. Silica-based devices have been at the forefront of such innovations for their ability to support optical excitations persisting for nearly 1 billion cycles, and for their low optical nonlinearity. While acoustic phonon modes can persist for a similar number of cycles in crystalline solids at cryogenic temperatures, it has not been possible to achieve such performance in silica, as silica becomes acoustically opaque at low temperatures. We demonstrate that these intrinsic forms of phonon dissipation are greatly reduced (by >90%) by nonlinear saturation using continuous drive fields of disparate frequencies. The result is a form of steady-state phononic spectral hole burning that produces a wideband transparency window with optically generated phonon fields of modest (nW) powers. We developed a simple model that explains both dissipative and dispersive changes produced by phononic saturation. Our studies, conducted in a microscale device, represent an important step towards engineerable phonon dynamics on demand and the use of glasses as low-loss phononic media.

  6. High-Q cross-plate phononic crystal resonator for enhanced acoustic wave localization and energy harvesting

    NASA Astrophysics Data System (ADS)

    Yang, Aichao; Li, Ping; Wen, Yumei; Yang, Chao; Wang, Decai; Zhang, Feng; Zhang, Jiajia

    2015-05-01

    A high-Q cross-plate phononic crystal resonator (Cr-PCR) coupled with an electromechanical Helmholtz resonator (EMHR) is proposed to improve acoustic wave localization and energy harvesting. Owing to the strongly directional wave-scattering effect of the cross-plate corners, strong confinement of acoustic waves emerges. Consequently, the proposed Cr-PCR structure exhibits ∼353.5 times higher Q value and ∼6.1 times greater maximum pressure amplification than the phononic crystal resonator (Cy-PCR) (consisting of cylindrical scatterers) of the same size. Furthermore, the harvester using the proposed Cr-PCR and the EMHR has ∼22 times greater maximum output-power volume density than the previous harvester using Cy-PCR and EMHR structures.

  7. Intervalley scattering by acoustic phonons in two-dimensional MoS2 revealed by double-resonance Raman spectroscopy.

    PubMed

    Carvalho, Bruno R; Wang, Yuanxi; Mignuzzi, Sandro; Roy, Debdulal; Terrones, Mauricio; Fantini, Cristiano; Crespi, Vincent H; Malard, Leandro M; Pimenta, Marcos A

    2017-03-09

    Double-resonance Raman scattering is a sensitive probe to study the electron-phonon scattering pathways in crystals. For semiconducting two-dimensional transition-metal dichalcogenides, the double-resonance Raman process involves different valleys and phonons in the Brillouin zone, and it has not yet been fully understood. Here we present a multiple energy excitation Raman study in conjunction with density functional theory calculations that unveil the double-resonance Raman scattering process in monolayer and bulk MoS2. Results show that the frequency of some Raman features shifts when changing the excitation energy, and first-principle simulations confirm that such bands arise from distinct acoustic phonons, connecting different valley states. The double-resonance Raman process is affected by the indirect-to-direct bandgap transition, and a comparison of results in monolayer and bulk allows the assignment of each Raman feature near the M or K points of the Brillouin zone. Our work highlights the underlying physics of intervalley scattering of electrons by acoustic phonons, which is essential for valley depolarization in MoS2.

  8. Intervalley scattering by acoustic phonons in two-dimensional MoS2 revealed by double-resonance Raman spectroscopy

    PubMed Central

    Carvalho, Bruno R.; Wang, Yuanxi; Mignuzzi, Sandro; Roy, Debdulal; Terrones, Mauricio; Fantini, Cristiano; Crespi, Vincent H.; Malard, Leandro M.; Pimenta, Marcos A.

    2017-01-01

    Double-resonance Raman scattering is a sensitive probe to study the electron-phonon scattering pathways in crystals. For semiconducting two-dimensional transition-metal dichalcogenides, the double-resonance Raman process involves different valleys and phonons in the Brillouin zone, and it has not yet been fully understood. Here we present a multiple energy excitation Raman study in conjunction with density functional theory calculations that unveil the double-resonance Raman scattering process in monolayer and bulk MoS2. Results show that the frequency of some Raman features shifts when changing the excitation energy, and first-principle simulations confirm that such bands arise from distinct acoustic phonons, connecting different valley states. The double-resonance Raman process is affected by the indirect-to-direct bandgap transition, and a comparison of results in monolayer and bulk allows the assignment of each Raman feature near the M or K points of the Brillouin zone. Our work highlights the underlying physics of intervalley scattering of electrons by acoustic phonons, which is essential for valley depolarization in MoS2. PMID:28276472

  9. Intervalley scattering by acoustic phonons in two-dimensional MoS2 revealed by double-resonance Raman spectroscopy

    NASA Astrophysics Data System (ADS)

    Carvalho, Bruno R.; Wang, Yuanxi; Mignuzzi, Sandro; Roy, Debdulal; Terrones, Mauricio; Fantini, Cristiano; Crespi, Vincent H.; Malard, Leandro M.; Pimenta, Marcos A.

    2017-03-01

    Double-resonance Raman scattering is a sensitive probe to study the electron-phonon scattering pathways in crystals. For semiconducting two-dimensional transition-metal dichalcogenides, the double-resonance Raman process involves different valleys and phonons in the Brillouin zone, and it has not yet been fully understood. Here we present a multiple energy excitation Raman study in conjunction with density functional theory calculations that unveil the double-resonance Raman scattering process in monolayer and bulk MoS2. Results show that the frequency of some Raman features shifts when changing the excitation energy, and first-principle simulations confirm that such bands arise from distinct acoustic phonons, connecting different valley states. The double-resonance Raman process is affected by the indirect-to-direct bandgap transition, and a comparison of results in monolayer and bulk allows the assignment of each Raman feature near the M or K points of the Brillouin zone. Our work highlights the underlying physics of intervalley scattering of electrons by acoustic phonons, which is essential for valley depolarization in MoS2.

  10. Wide-Stopband Aperiodic Phononic Filters

    NASA Technical Reports Server (NTRS)

    Rostem, Karwan; Chuss, David; Denis, K. L.; Wollack, E. J.

    2016-01-01

    We demonstrate that a phonon stopband can be synthesized from an aperiodic structure comprising a discrete set of phononic filter stages. Each element of the set has a dispersion relation that defines a complete bandgap when calculated under a Bloch boundary condition. Hence, the effective stopband width in an aperiodic phononic filter (PnF) may readily exceed that of a phononic crystal with a single lattice constant or a coherence scale. With simulations of multi-moded phononic waveguides, we discuss the effects of finite geometry and mode-converting junctions on the phonon transmission in PnFs. The principles described may be utilized to form a wide stopband in acoustic and surface wave media. Relative to the quantum of thermal conductance for a uniform mesoscopic beam, a PnF with a stopband covering 1.6-10.4 GHz is estimated to reduce the thermal conductance by an order of magnitude at 75 mK.

  11. A fractional calculus model of anomalous dispersion of acoustic waves.

    PubMed

    Wharmby, Andrew W

    2016-09-01

    An empirical formula based on viscoelastic analysis techniques that employs concepts from the fractional calculus that was used to model the dielectric behavior of materials exposed to oscillating electromagnetic fields in the radiofrequency, terahertz, and infrared bands. This work adapts and applies the formula to model viscoelastic behavior of materials that show an apparent increase of phase velocity of vibration with an increase in frequency, otherwise known as anomalous dispersion. A fractional order wave equation is derived through the application of the classic elastic-viscoelastic correspondence principle whose analytical solution is used to describe absorption and dispersion of acoustic waves in the viscoelastic material displaying anomalous dispersion in a specific frequency range. A brief discussion and comparison of an alternative fractional order wave equation recently formulated is also included.

  12. Modelling of acoustic waves propagating in nesting Fibonacci super-lattice phononic crystal

    NASA Astrophysics Data System (ADS)

    Zhao, Min; Qi, Hai-Feng; Xu, Jia-Hui; Xie, Ya-Zhuo; Zhang, Xing-Gan; Gao, Jian

    2014-07-01

    Herein, we report construction of one kind of nesting-Fibonacci-super-lattice phononic crystal, in which the super-lattice cell is a well-defined Fibonacci generation sequence. We present a comparative study on band-gap structures of acoustic waves propagating in one-dimensional, nesting Fibonacci-periodic structure and simple-periodic structure. We find that there are more band gaps in nesting Fibonacci super-lattice models, and that they present behavior different from the split-up of band gaps with different generation numbers. With the increase of generation number, more band gaps split and occur. Additionally, when generation number becomes larger, Bragg scattering becomes more significant: the characteristic curves become flatter and band gaps become wider. Furthermore, we study the effect of various parameters such as density, thickness and defects on band-gap structures. Our work is significant both for understanding the intrinsic physical properties of nesting Fibonacci sequences and for providing flexible choices to meet real engineering requirements.

  13. Phonons in twisted bilayer graphene

    NASA Astrophysics Data System (ADS)

    Cocemasov, Alexandr I.; Nika, Denis L.; Balandin, Alexander A.

    2013-07-01

    We theoretically investigate phonon dispersion in AA-stacked, AB-stacked, and twisted bilayer graphene with various rotation angles. The calculations are performed using the Born-von Karman model for the intralayer atomic interactions and the Lennard-Jones potential for the interlayer interactions. It is found that the stacking order affects the out-of-plane acoustic phonon modes the most. The difference in the phonon densities of states in the twisted bilayer graphene and in AA- or AB-stacked bilayer graphene appears in the phonon frequency range 90-110 cm-1. Twisting bilayer graphene leads to the emergence of different phonon branches—termed hybrid folded phonons—which originate from the mixing of phonon modes from different high-symmetry directions in the Brillouin zone. The frequencies of the hybrid folded phonons depend strongly on the rotation angle and can be used for noncontact identification of the twist angles in graphene samples. The obtained results and the tabulated frequencies of phonons in twisted bilayer graphene are important for the interpretation of experimental Raman data and in determining the thermal conductivity of these material systems.

  14. Coherent acoustic phonons in YBa2Cu3O7/La1/3Ca2/3MnO3 superlattices

    NASA Astrophysics Data System (ADS)

    Li, Wei; He, Bin; Zhang, Chunfeng; Liu, Shenghua; Liu, Xiaoran; Middey, S.; Chakhalian, J.; Wang, Xiaoyong; Xiao, Min

    2016-03-01

    We investigate photo-induced coherent acoustic phonons in complex oxide superlattices consisting of high-Tc superconductor YBa2Cu3O7-x and ferromagnetic manganite La1/3Ca2/3MnO3 epitaxial layers with broadband pump-probe spectroscopy. Two oscillatory components have been observed in time-resolved differential reflectivity spectra. Based on the analysis, the slow oscillation mode with a frequency sensitive to the probe wavelength is ascribed to the stimulated Brillouin scattering due to the photon reflection by propagating train of coherent phonons. The fast oscillation mode with a probe-wavelength-insensitive frequency is attributed to the Bragg oscillations caused by specular phonon reflections at oxide interfaces or the electron-coupling induced modulation due to free carrier absorption in the metallic superlattices. Our findings suggest that oxide superlattice is an ideal system to tailor the coherent behaviors of acoustic phonons and to manipulate the thermal and acoustic properties.

  15. AB INITIO STUDY OF PHONON DISPERSION AND ELASTIC PROPERTIES OF L12 INTERMETALLICS Ti3Al AND Y3Al

    NASA Astrophysics Data System (ADS)

    Arikan, N.; Ersen, M.; Ocak, H. Y.; Iyigör, A.; Candan, A.; UǦUR, Ş.; UǦUR, G.; Khenata, R.; Varshney, D.

    2013-12-01

    In this paper, the structural, elastic and phonon properties of Ti3Al and Y3Al in L12(Cu3Al) phase are studied by performing first-principles calculations within the generalized gradient approximation. The calculated lattice constants, static bulk moduli, first-order pressure derivative of bulk moduli and elastic constants for both compounds are reported. The phonon dispersion curves along several high-symmetry lines at the Brillouin zone, together with the corresponding phonon density of states, are determined using the first-principles linear-response approach of the density functional perturbation theory. Temperature variations of specific heat in the range of 0-500 K are obtained using the quasi-harmonic model.

  16. Lattice dynamics of xenotime: The phonon dispersion relations and density of states of LuPO{sub 4}

    SciTech Connect

    Nipko, J.C.; Loong, C.; Loewenhaupt, M.; Braden, M.; Reichardt, W.; Boatner, L.A.

    1997-11-01

    LuPO{sub 4} is the nonmagnetic end member of a series of rare-earth phosphates with a common zircon-type crystal structure. The phonon-dispersion curves of LuPO{sub 4} along the [x,0,0], [x,x,0], and [0,0,x] symmetry directions were measured by neutron triple-axis spectroscopy using single-crystal samples. The phonon density of states was determined by time-of-flight neutron scattering using polycrystalline samples. Phonons involving mainly motions of rare-earth ions were found to be well separated in energy from those of the P and O vibrations. A large gap in the phonon-frequency-distribution function, which divides the O-P-O bending-type motions from the P-O stretches, was observed. All of the experimental results were satisfactorily accounted for by lattice-dynamic shell-model calculations. LuPO{sub 4} is a host material for the incorporation of rare-earth ions to produce activated luminescence. Information regarding the phonon and thermodynamic properties of LuPO{sub 4} is pertinent to extended investigations of additional rare-earth spin-lattice interactions in other zircon-structure rare-earth orthophosphates. {copyright} {ital 1997} {ital The American Physical Society}

  17. Strong Amplification of Coherent Acoustic Phonons by Intraminiband Currents in a Semiconductor Superlattice

    NASA Astrophysics Data System (ADS)

    Shinokita, Keisuke; Reimann, Klaus; Woerner, Michael; Elsaesser, Thomas; Hey, Rudolf; Flytzanis, Christos

    2016-02-01

    Sound amplification in an electrically biased superlattice (SL) is studied in optical experiments with 100 fs time resolution. Coherent SL phonons with frequencies of 40, 375, and 410 GHz give rise to oscillatory reflectivity changes. With currents from 0.5 to 1.3 A, the Fourier amplitude of the 410 GHz phonon increases by more than a factor of 2 over a 200 ps period. This amplification is due to stimulated Čerenkov phonon emission by electrons undergoing intraminiband transport. The gain coefficient of 8 ×103 cm-1 is reproduced by theoretical calculations and holds potential for novel sub-THz phonon emitters.

  18. Acoustic-phonon-assisted quantum control of qubit states near the Si/SiO2 interface

    NASA Astrophysics Data System (ADS)

    Gou, Bing-Ping; Zhao, Peiji; Kong, Xiao-Jun

    2013-10-01

    The waiting time between load/initialization and readout of electron spin qubit is related to electron tunneling between the donor and Si/SiO2 interface. Impacts of energy valley interference in silicon, lattice temperature, and screening of metallic gate on the waiting time associated with acoustic-phonon-assisted electron tunneling have been investigated. The results show that interface valley-orbit coupling causes its oscillation with donor depth and the influence of gate screening is significant when the SiO2 thickness is smaller than 10 nm. Moreover, the influences of these factors are strongest at critical electric field.

  19. Quantitative Determination of Lateral Mode Dispersion in Film Bulk Acoustic Resonators through Laser Acoustic Imaging

    SciTech Connect

    Ken Telschow; John D. Larson III

    2006-10-01

    Film Bulk Acoustic Resonators are useful for many signal processing applications. Detailed knowledge of their operation properties are needed to optimize their design for specific applications. The finite size of these resonators precludes their use in single acoustic modes; rather, multiple wave modes, such as, lateral wave modes are always excited concurrently. In order to determine the contributions of these modes, we have been using a newly developed full-field laser acoustic imaging approach to directly measure their amplitude and phase throughout the resonator. This paper describes new results comparing modeling of both elastic and piezoelectric effects in the active material with imaging measurement of all excited modes. Fourier transformation of the acoustic amplitude and phase displacement images provides a quantitative determination of excited mode amplitude and wavenumber at any frequency. Images combined at several frequencies form a direct visualization of lateral mode excitation and dispersion for the device under test allowing mode identification and comparison with predicted operational properties. Discussion and analysis are presented for modes near the first longitudinal thickness resonance (~900 MHz) in an AlN thin film resonator. Plate wave modeling, taking account of material crystalline orientation, elastic and piezoelectric properties and overlayer metallic films, will be discussed in relation to direct image measurements.

  20. Strong Amplification of Coherent Acoustic Phonons by Intraminiband Currents in a Semiconductor Superlattice.

    PubMed

    Shinokita, Keisuke; Reimann, Klaus; Woerner, Michael; Elsaesser, Thomas; Hey, Rudolf; Flytzanis, Christos

    2016-02-19

    Sound amplification in an electrically biased superlattice (SL) is studied in optical experiments with 100 fs time resolution. Coherent SL phonons with frequencies of 40, 375, and 410 GHz give rise to oscillatory reflectivity changes. With currents from 0.5 to 1.3 A, the Fourier amplitude of the 410 GHz phonon increases by more than a factor of 2 over a 200 ps period. This amplification is due to stimulated Čerenkov phonon emission by electrons undergoing intraminiband transport. The gain coefficient of 8×10^{3}  cm^{-1} is reproduced by theoretical calculations and holds potential for novel sub-THz phonon emitters.

  1. Hypersonic phonon propagation in one-dimensional surface phononic crystal

    NASA Astrophysics Data System (ADS)

    Graczykowski, B.; Sledzinska, M.; Kehagias, N.; Alzina, F.; Reparaz, J. S.; Sotomayor Torres, C. M.

    2014-03-01

    Hypersonic, thermally activated surface acoustic waves propagating in the surface of crystalline silicon patterned with periodic stripes were studied by Brillouin light scattering. Two characteristic directions (normal and parallel to the stripes) of surface acoustic waves propagation were examined exhibiting a distinctive propagation behavior. The measured phononic band structure exhibits diverse features, such as zone folding, band gap opening, and hybridization to local resonance for waves propagating normal to the stripes, and a variety of dispersive modes propagating along the stripes. Experimental results were supported by theoretical calculations performed using finite element method.

  2. A new approach to measure phonon dispersion relation (PDR) by Raman scattering and a downbending observation in diamond PDR

    NASA Astrophysics Data System (ADS)

    Zhang, Shu-Lin; Xia, Lei; Chen, Weihua; Li, D. Y.; Li, Wanyu; He, Juan

    2016-12-01

    The phonon dispersion relation (PDR), i.e., the dependence of phonon frequency ω on its wavevector q, ω(q), was measured traditionally by inelastic neutron scattering (INS) or inelastic X-ray scattering (IXS). A new approach to measure PDR by Raman scattering (RS) of nanostructures was proposed and applied to observe the longitudinal optical (LO) PDR of diamond successfully. Due to the higher resolution and accuracy of ω and q in RS, a clear downbending feature of ω with increasing q away from the Brillouin zoon center was observed for the first time. The validity of the new approach has been confirmed also by the appearing of the downward bending in PDR, which is originally measured by traditional high-resolution IXS experiment. The downbending feature may give us a clue for deep understanding of the interactions occur in diamond, while the overbending feature observed by INS and IXS has been attributed to strong effective second-nearest-neighbor forces.

  3. Phonon dynamics of graphene on metals

    NASA Astrophysics Data System (ADS)

    Taleb, Amjad Al; Farías, Daniel

    2016-03-01

    The study of surface phonon dispersion curves is motivated by the quest for a detailed understanding of the forces between the atoms at the surface and in the bulk. In the case of graphene, additional motivation comes from the fact that thermal conductivity is dominated by contributions from acoustic phonons, while optical phonon properties are essential to understand Raman spectra. In this article, we review recent progress made in the experimental determination of phonon dispersion curves of graphene grown on several single-crystal metal surfaces. The two main experimental techniques usually employed are high-resolution electron energy loss spectroscopy (HREELS) and inelastic helium atom scattering (HAS). The different dispersion branches provide a detailed insight into the graphene-substrate interaction. Softening of optical modes and signatures of the substrate‧s Rayleigh wave are observed for strong graphene-substrate interactions, while acoustic phonon modes resemble those of free-standing graphene for weakly interacting systems. The latter allows determining the bending rigidity and the graphene-substrate coupling strength. A comparison between theory and experiment is discussed for several illustrative examples. Perspectives for future experiments are discussed.

  4. Acoustic phonon-limited diffusion thermopower in monolayer MoS{sub 2}

    SciTech Connect

    Patil, S. B.; Sankeshwar, N. S. Kubakaddi, S. S.

    2015-06-24

    Diffusion thermopower S{sub d} is investigated, theoretically, as a function of temperature, T and electron concentration, n{sub s} in a n-type monolayer molebdenum disulfide (MoS{sub 2}). Electron scattering due to unscreened deformation potential (DP) coupling of TA phonons, screened DP coupling of LA phonons, and screened piezoelectric (PE) coupling of LA and TA phonons is considered. Total S{sub d} is dominated by electron scattering by TA phonons via unscreened DP coupling. S{sub d} is found to increase (decrease) with increasing T (n{sub s}). At low T and for high n{sub s}, S{sub d} ∼ T and n{sub s}{sup −1} as found from the Mott formula. At a given T and for given ns, S{sub d} in MoS{sub 2} is much larger than that in GaAs, due to the larger electron effective mass in the former.

  5. Strong Energy-momentum Dispersion of Phonon Dressed Carriers in the Lightly Doped Band Insulator SrTiO3

    SciTech Connect

    Meevasana, Warawat

    2010-05-26

    Much progress has been made recently in the study of the effects of electron-phonon (el-ph) coupling in doped insulators using angle resolved photoemission (ARPES), yielding evidence for the dominant role of el-ph interactions in underdoped cuprates. As these studies have been limited to doped Mott insulators, the important question arises how this compares with doped band insulators where similar el-ph couplings should be at work. The archetypical case is the perovskite SrTiO{sub 3} (STO), well known for its giant dielectric constant of 10000 at low temperature, exceeding that of La{sub 2}CuO{sub 4} by a factor of 500. Based on this fact, it has been suggested that doped STO should be the archetypical bipolaron superconductor. Here we report an ARPES study from high-quality surfaces of lightly doped SrTiO{sub 3}. Comparing to lightly doped Mott insulators, we find the signatures of only moderate electron-phonon coupling: a dispersion anomaly associated with the low frequency optical phonon with a {lambda}{prime} {approx} 0.3 and an overall bandwidth renormalization suggesting an overall {lambda}{prime} {approx} 0.7 coming from the higher frequency phonons. Further, we find no clear signatures of the large pseudogap or small polaron phenomena. These findings demonstrate that a large dielectric constant itself is not a good indicator of el-ph coupling and highlight the unusually strong effects of the el-ph coupling in doped Mott insulators.

  6. Ultrafast dynamics of quasiparticles and coherent acoustic phonons in slightly underdoped (BaK)Fe2As2

    PubMed Central

    Lin, Kung-Hsuan; Wang, Kuan-Jen; Chang, Chung-Chieh; Wen, Yu-Chieh; Lv, Bing; Chu, Ching-Wu; Wu, Maw-Kuen

    2016-01-01

    We have utilized ultrafast optical spectroscopy to study carrier dynamics in slightly underdoped (BaK)Fe2As2 crystals without magnetic transition. The photoelastic signals due to coherent acoustic phonons have been quantitatively investigated. According to our temperature-dependent results, we found that the relaxation component of superconducting quasiparticles persisted from the superconducting state up to at least 70 K in the normal state. Our findings suggest that the pseudogaplike feature in the normal state is possibly the precursor of superconductivity. We also highlight that the pseudogap feature of K-doped BaFe2As2 is different from that of other iron-based superconductors, including Co-doped or P-doped BaFe2As2. PMID:27180873

  7. Detecting the Photoexcited Carrier Distribution Across GaAs/Transition Metal Oxide Interfaces by Coherent Longitudinal Acoustic Phonons.

    PubMed

    Pollock, Kevin L; Doan, Hoang Q; Rustagi, Avinash; Stanton, Christopher J; Cuk, Tanja

    2017-03-02

    A prominent architecture for solar energy conversion layers diverse materials, such as traditional semiconductors (Si, III-V) and transition metal oxides (TMOs), into a monolithic device. The efficiency with which photoexcited carriers cross each layer is critical to device performance and dependent on the electronic properties of a heterojunction. Here, by time-resolved changes in the reflectivity after excitation of an n-GaAs/p-GaAs/TMO (Co3O4, IrO2) device, we detect a photoexcited carrier distribution specific to the p-GaAs/TMO interface through its coupling to phonons in both materials. The photoexcited carriers generate two coherent longitudinal acoustic phonons (CLAPs) traveling in opposite directions, one into the TMO and the other into the p-GaAs. This is the first time a CLAP is reported to originate at a semiconductor/TMO heterojunction. Therefore, these experiments seed future modeling of the built-in electric fields, the internal Fermi level, and the photoexcited carrier density of semiconductor/TMO interfaces within multilayered heterostructures.

  8. Time domain characteristics of wave motion in dispersive and anisotropic continuum acoustic metamaterials.

    PubMed

    Wang, Zhaojun; Zhou, Xiaoming

    2016-12-01

    The authors study the wave propagation in continuum acoustic metamaterials whose all or not all of the principal elements of the mass tensor or the scalar compressibility can be negative due to wave dispersion. Their time-domain wave characteristics are particularly investigated by the finite-difference time-domain (FDTD) method, in which algorithms for the Drude and Lorentz dispersion pertinent to acoustic metamaterials are provided necessarily. Wave propagation nature of anisotropic acoustic metamaterials with all admissible material parameters are analyzed in a general manner. It is found that anomalous negative refraction phenomena can appear in several dispersion regimes, and their unique time-domain signatures have been discovered by the FDTD modeling. It is further proposed that two different metamaterial layers with specially assigned dispersions could comprise a conjugate pair that permits wave propagation only at specific points in the wave vector space. The time-domain pulse simulation verifies that acoustic directive radiation capable of modulating radiation angle with the wave frequency can be realized with this conjugate pair. The study provides the detailed analysis of wave propagation in anisotropic and dispersive acoustic mediums, which makes a further step toward dispersion engineering and transient wave control through acoustic metamaterials.

  9. Tunable broadband unidirectional acoustic transmission based on a waveguide with phononic crystal

    NASA Astrophysics Data System (ADS)

    Song, Ailing; Chen, Tianning; Wang, Xiaopeng; Wan, Lele

    2016-08-01

    In this paper, a tunable broadband unidirectional acoustic transmission (UAT) device composed of a bended tube and a superlattice with square columns is proposed and numerically investigated by using finite element method. The UAT is realized in the proposed UAT device within two wide frequency ranges. And the effectiveness of the UAT device is demonstrated by analyzing the sound pressure distributions when the acoustic waves are incident from different directions. The unidirectional band gaps can be effectively tuned by mechanically rotating the square columns, which is a highlight of this paper. Besides, a bidirectional acoustic isolation (BAI) device is obtained by placing two superlattices in the bended tube, in which the acoustic waves cannot propagate along any directions. The physical mechanisms of the proposed UAT device and BAI device are simply discussed. The proposed models show potential applications in some areas, such as unidirectional sonic barrier or noise insulation.

  10. Significant reduction of lattice thermal conductivity due to phonon confinement in graphene nanoribbons

    NASA Astrophysics Data System (ADS)

    Nissimagoudar, A. S.; Sankeshwar, N. S.

    2014-06-01

    Lattice thermal conductivity, κp, of suspended and supported graphene nanoribbons (GNRs) is studied over a wide temperature range, taking into account the dispersive nature of confined acoustic phonon modes. Employing a modified Callaway model, an expression for κp is developed, considering the explicit contributions from in-plane longitudinal, transverse, and torsional acoustic, and out-of-plane flexural acoustic phonon modes. Numerical calculations of κp(T) are presented assuming the confined acoustic phonons to be scattered by sample boundaries, impurities, and other phonons via both normal and umklapp processes. The effect of phonon confinement is to modify the phonon group velocities and the temperature dependence of κp. In a suspended 5-nm-wide GNR at room temperature, a decrease in κp by ˜70% is predicted. Our study brings out the relative importance of the contributing phonon modes and reveals the influence of flexural phonons on κp as a marked shoulder at low temperatures. The role of the various sample-dependent scattering mechanisms is examined. The substrate, in supported GNRs, is shown to curtail the phonon mean free path and suppress the low-temperature κp. Our results are in good agreement with recent experimental data of Bae et al. [M. H. Bae, Z. Li, Z. Aksamija, P. N. Martin, F. Xiong, Z. Y. Ong, I. Knezevic, and E. Pop, Nat. Commun. 4, 1734 (2013), 10.1038/ncomms2755] for supported GNRs.

  11. Dispersion relations of elastic waves in one-dimensional piezoelectric/piezomagnetic phononic crystal with functionally graded interlayers.

    PubMed

    Guo, Xiao; Wei, Peijun; Lan, Man; Li, Li

    2016-08-01

    The effects of functionally graded interlayers on dispersion relations of elastic waves in a one-dimensional piezoelectric/piezomagnetic phononic crystal are studied in this paper. First, the state transfer equation of the functionally graded interlayer is derived from the motion equation by the reduction of order (from second order to first order). The transfer matrix of the functionally graded interlayer is obtained by solving the state transfer equation with the spatial-varying coefficient. Based on the transfer matrixes of the piezoelectric slab, the piezomagnetic slab and the functionally graded interlayers, the total transfer matrix of a single cell is obtained. Further, the Bloch theorem is used to obtain the resultant dispersion equations of in-plane and anti-plane Bloch waves. The dispersion equations are solved numerically and the numerical results are shown graphically. Five kinds of profiles of functionally graded interlayers between a piezoelectric slab and a piezomagnetic slab are considered. It is shown that the functionally graded interlayers have evident influences on the dispersion curves and the band gaps.

  12. Physically founded phonon dispersions of few-layer materials and the case of borophene

    DOE PAGES

    Carrete, Jesús; Li, Wu; Lindsay, Lucas; ...

    2016-04-21

    By building physically sound interatomic force constants,we offer evidence of the universal presence of a quadratic phonon branch in all unstrained 2D materials, thus contradicting much of the existing literature. Through a reformulation of the interatomic force constants (IFCs) in terms of internal coordinates, we find that a delicate balance between the IFCs is responsible for this quadraticity. We use this approach to predict the thermal conductivity of Pmmn borophene, which is comparable to that of MoS2, and displays a remarkable in-plane anisotropy. Ultimately, these qualities may enable the efficient heat management of borophene devices in potential nanoelectronic applications

  13. Physically founded phonon dispersions of few-layer materials and the case of borophene

    SciTech Connect

    Carrete, Jesús; Li, Wu; Lindsay, Lucas; Broido, David A.; Gallego, Luis J.; Mingo, Natalio

    2016-04-21

    By building physically sound interatomic force constants,we offer evidence of the universal presence of a quadratic phonon branch in all unstrained 2D materials, thus contradicting much of the existing literature. Through a reformulation of the interatomic force constants (IFCs) in terms of internal coordinates, we find that a delicate balance between the IFCs is responsible for this quadraticity. We use this approach to predict the thermal conductivity of Pmmn borophene, which is comparable to that of MoS2, and displays a remarkable in-plane anisotropy. Ultimately, these qualities may enable the efficient heat management of borophene devices in potential nanoelectronic applications

  14. Phonon dispersion relation of Mg-Cu-Gd bulk metallic glasses

    NASA Astrophysics Data System (ADS)

    Suthar, P. H.

    2016-05-01

    Collective dynamics and elastic constants of bulk metallic glasses Mg65Cu25Gd10 and Mg60Cu25Gd15 are computed using the Hubbard -Beeby approach and our well recognized model potential. The important ingredients in the present study are the pair potential and local field correction functions (LFCF). The local field correction functions due to Hartree (H), Farid et al (F) and Sarkar Sen et al (S) are employed to investigation the influence of the screening effects on the longitudinal and traversed of phonon modes of glassy system. The results for the elastic constants are found to be in good agreement with experimental data.

  15. Surface phononic graphene

    NASA Astrophysics Data System (ADS)

    Yu, Si-Yuan; Sun, Xiao-Chen; Ni, Xu; Wang, Qing; Yan, Xue-Jun; He, Cheng; Liu, Xiao-Ping; Feng, Liang; Lu, Ming-Hui; Chen, Yan-Feng

    2016-12-01

    Strategic manipulation of wave and particle transport in various media is the key driving force for modern information processing and communication. In a strongly scattering medium, waves and particles exhibit versatile transport characteristics such as localization, tunnelling with exponential decay, ballistic, and diffusion behaviours due to dynamical multiple scattering from strong scatters or impurities. Recent investigations of graphene have offered a unique approach, from a quantum point of view, to design the dispersion of electrons on demand, enabling relativistic massless Dirac quasiparticles, and thus inducing low-loss transport either ballistically or diffusively. Here, we report an experimental demonstration of an artificial phononic graphene tailored for surface phonons on a LiNbO3 integrated platform. The system exhibits Dirac quasiparticle-like transport, that is, pseudo-diffusion at the Dirac point, which gives rise to a thickness-independent temporal beating for transmitted pulses, an analogue of Zitterbewegung effects. The demonstrated fully integrated artificial phononic graphene platform here constitutes a step towards on-chip quantum simulators of graphene and unique monolithic electro-acoustic integrated circuits.

  16. Surface phononic graphene.

    PubMed

    Yu, Si-Yuan; Sun, Xiao-Chen; Ni, Xu; Wang, Qing; Yan, Xue-Jun; He, Cheng; Liu, Xiao-Ping; Feng, Liang; Lu, Ming-Hui; Chen, Yan-Feng

    2016-12-01

    Strategic manipulation of wave and particle transport in various media is the key driving force for modern information processing and communication. In a strongly scattering medium, waves and particles exhibit versatile transport characteristics such as localization, tunnelling with exponential decay, ballistic, and diffusion behaviours due to dynamical multiple scattering from strong scatters or impurities. Recent investigations of graphene have offered a unique approach, from a quantum point of view, to design the dispersion of electrons on demand, enabling relativistic massless Dirac quasiparticles, and thus inducing low-loss transport either ballistically or diffusively. Here, we report an experimental demonstration of an artificial phononic graphene tailored for surface phonons on a LiNbO3 integrated platform. The system exhibits Dirac quasiparticle-like transport, that is, pseudo-diffusion at the Dirac point, which gives rise to a thickness-independent temporal beating for transmitted pulses, an analogue of Zitterbewegung effects. The demonstrated fully integrated artificial phononic graphene platform here constitutes a step towards on-chip quantum simulators of graphene and unique monolithic electro-acoustic integrated circuits.

  17. Phononic crystal surface mode coupling and its use in acoustic Doppler velocimetry.

    PubMed

    Cicek, Ahmet; Salman, Aysevil; Kaya, Olgun Adem; Ulug, Bulent

    2016-02-01

    It is numerically shown that surface modes of two-dimensional phononic crystals, which are Bloch modes bound to the interface between the phononic crystal and the surrounding host, can couple back and forth between the surfaces in a length scale determined by the separation of two surfaces and frequency. Supercell band structure computations through the finite-element method reveal that the surface band of an isolated surface splits into two bands which support either symmetric or antisymmetric hybrid modes. When the surface separation is 3.5 times the lattice constant, a coupling length varying between 30 and 48 periods can be obtained which first increases linearly with frequency and, then, decreases rapidly. In the linear regime, variation of coupling length can be used as a means of measuring speeds of objects on the order of 0.1m/s by incorporating the Doppler shift. Speed sensitivity can be improved by increasing surface separation at the cost of larger device sizes.

  18. Phonon dispersions and Fermi surfaces nesting explaining the variety of charge ordering in titanium-oxypnictides superconductors

    PubMed Central

    Nakano, Kousuke; Hongo, Kenta; Maezono, Ryo

    2016-01-01

    There has been a puzzle between experiments and theoretical predictions on the charge ordering of layered titanium-oxypnictides superconductors. Unconventional mechanisms to explain this discrepancy have been argued so far, even affecting the understanding of superconductivity on the compound. We provide a new theoretical prediction, by which the discrepancy itself is resolved without any complicated unconventional explanation. Phonon dispersions and changes of nesting vectors in Fermi surfaces are clarified to lead to the variety of superlattice structures even for the common crystal structures when without CDW, including orthorhombic 2 × 2 × 1 one for BaTi2As2O, which has not yet been explained successfully so far, being different from tetragonal for BaTi2Sb2O and BaTi2Bi2O. The electronic structure analysis can naturally explain experimental observations about CDW including most latest ones without any cramped unconventional mechanisms. PMID:27430418

  19. Cross-plane heat conduction in thin films with ab-initio phonon dispersions and scattering rates

    NASA Astrophysics Data System (ADS)

    Vermeersch, Bjorn; Carrete, Jesús; Mingo, Natalio

    2016-05-01

    We present a first-principles study of the cross-plane thermal conductivity κ ⊥ in a wide variety of semiconductor thin films. We introduce a simple suppression model that matches variance-reduced Monte Carlo simulations with ab-initio phonon dispersions and scattering rates within ≤ 5 % even for anisotropic compounds. This, in turn, enables accurate κ ⊥ reconstruction from tabulated cumulative conductivity curves κ Σ ( Λ ⊥ ) . We furthermore reveal, and explain, a distinct quasiballistic regime characterised by a fractional thickness dependence κ ⊥ ˜ L 2 - α in alloys (where α is the Lévy exponent) and logarithmic dependence κ ⊥ ˜ ln ( L ) in single crystals. These observations culminate in the formulation of two compact parametric forms for κ ⊥ ( L ) that can fit the first-principles curves across the entire ballistic-diffusive range within a few percent for all investigated compounds.

  20. Electron-phonon interaction model and prediction of thermal energy transport in SOI transistor.

    PubMed

    Jin, Jae Sik; Lee, Joon Sik

    2007-11-01

    An electron-phonon interaction model is proposed and applied to thermal transport in semiconductors at micro/nanoscales. The high electron energy induced by the electric field in a transistor is transferred to the phonon system through electron-phonon interaction in the high field region of the transistor. Due to this fact, a hot spot occurs, which is much smaller than the phonon mean free path in the Si-layer. The full phonon dispersion model based on the Boltzmann transport equation (BTE) with the relaxation time approximation is applied for the interactions among different phonon branches and different phonon frequencies. The Joule heating by the electron-phonon scattering is modeled through the intervalley and intravalley processes for silicon by introducing average electron energy. The simulation results are compared with those obtained by the full phonon dispersion model which treats the electron-phonon scattering as a volumetric heat source. The comparison shows that the peak temperature in the hot spot region is considerably higher and more localized than the previous results. The thermal characteristics of each phonon mode are useful to explain the above phenomena. The optical mode phonons of negligible group velocity obtain the highest energy density from electrons, and resides in the hot spot region without any contribution to heat transport, which results in a higher temperature in that region. Since the acoustic phonons with low group velocity show the higher energy density after electron-phonon scattering, they induce more localized heating near the hot spot region. The ballistic features are strongly observed when phonon-phonon scattering rates are lower than 4 x 10(10) S(-1).

  1. Tuning of acoustic wave dispersion in ferroelectrics—A theoretical study

    NASA Astrophysics Data System (ADS)

    Chang, Wontae

    2017-02-01

    Tuning of acoustic wave dispersion in ferroelectrics due to its electrostrictive effect is theoretically investigated. As the acoustic wave is excited electrically in ferroelectrics, the elastic stiffness tensor can be modified by both the linear piezoelectric and nonlinear electrostrictive electromechanical couplings depending on the wave excitation direction of the crystal, where the linear piezoelectric modification has been well characterized and extensively used for the application of piezoelectric-based acoustic wave devices over the past 50 years, but the nonlinear electrostrictive modification, determining the tuning of acoustic wave dispersion in the medium, is still too premature to use the properties in application. For the tuning application, it is essential to know how the electrostrictive strain actually tunes the propagation and displacement of the ferroelectrically active acoustic waves, and this information is currently unavailable. In this paper, the ferroelectrically active acoustic wave propagation and displacement in conjunction with the nonlinear electrostrictive modification are calculated using the plane wave expansion method, and the tunable wave properties associated with the propagation and displacement, are discussed. The electrically excited acoustic wave properties in ferroelectrics are largely modified from the electrostrictive effect, e.g., tuned, excited, vanished, coupled, decoupled, etc., and this should be taken into account in the development of ferroelectric-based acoustic wave devices.

  2. Phonons in Ge nanowires

    NASA Astrophysics Data System (ADS)

    Peelaers, H.; Partoens, B.; Peeters, F. M.

    2009-09-01

    The phonon spectra of thin freestanding, hydrogen passivated, Ge nanowires are calculated by ab initio techniques. The effect of confinement on the phonon modes as caused by the small diameters of the wires is investigated. Confinement causes a hardening of the optical modes and a softening of the longitudinal acoustic modes. The stability of the nanowires, undoped or doped with B or P atoms, is investigated using the obtained phonon spectra. All considered wires were stable, except for highly doped, very thin nanowires.

  3. Phononic crystals of poroelastic spheres

    NASA Astrophysics Data System (ADS)

    Alevizaki, A.; Sainidou, R.; Rembert, P.; Morvan, B.; Stefanou, N.

    2016-11-01

    An extension of the layer-multiple-scattering method to phononic crystals of poroelastic spheres immersed in a fluid medium is developed. The applicability of the method is demonstrated on specific examples of close-packed fcc crystals of submerged water-saturated meso- and macroporous silica microspheres. It is shown that, by varying the pore size and/or the porosity, the transmission, reflection, and absorption spectra of finite slabs of these crystals are significantly altered. Strong absorption, driven by the slow waves in the poroelastic material and enhanced by multiple scattering, leads to negligible transmittance over an extended frequency range, which might be useful for practical applications in broadband acoustic shielding. The results are analyzed by reference to relevant phononic dispersion diagrams in the viscous and inertial coupling limits, and a consistent interpretation of the underlying physics is provided.

  4. Phonon dispersion relations of Sb2S3 and Bi2S3 using the supercell force-constant method

    NASA Astrophysics Data System (ADS)

    Gan, Chee Kwan; Chua, Kun Ting Eddie; Liu, Yun

    2015-03-01

    We present a lattice dynamical study on the orthorhombic antimony sulphide (Sb2S3) and bismuth sulphide (Bi2S3) using the supercell force-constant method. We find that the slow decay of the interatomic force constants for these compounds in the Pnma setting critically demand the use of a large supercell of 2 × 4 × 2 that consists of 320 atoms. To enable a practical calculation the space group information is fully utilized where only inequivalent atoms within the primitive cell are displaced for the force calculations. The effect of Born effective charges is incorporated into the method. We compare our results with that obtained from the density-functional perturbation theory. We found that smaller supercells could lead to unphysical acoustic phonon softening and lifting of the degeneracies along high symmetry directions. Our results provide a proper guideline for the use of the supercell force-constant method: the supercell size must be carefully be tested along with other parameters such as the kinetic energy cutoff, the Brillouin zone sampling or the self-consistent convergence criteria.

  5. Holographically formed, acoustically switchable gratings based on polymer-dispersed liquid crystals.

    PubMed

    Liu, Yan Jun; Lu, Mengqian; Ding, Xiaoyun; Leong, Eunice S P; Lin, Sz-Chin Steven; Shi, Jinjie; Teng, Jing Hua; Wang, Lin; Bunning, Timothy J; Huang, Tony Jun

    2013-08-01

    We report holographic polymer-dispersed liquid crystal (H-PDLC) gratings driven by surface acoustic waves (SAWs). Our experiments show that upon applying SAWs, the H-PDLC grating exhibited switchable properties: The diffraction of the H-PDLC grating decreased, whereas the transmission increased. This acoustically switchable behavior is due to the acoustic streaming-induced realignment of liquid crystals as well as absorption-resulted thermal diffusion. Such SAW-driven H-PDLC gratings are potentially useful in many photonic applications, such as optical switches, spatial light modulators, and switchable add/drop filters.

  6. Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2

    DOE PAGES

    Gardner, D. R.; Bonnoit, C. J.; Chisnell, R.; ...

    2016-02-11

    In this paper, we study high-resolution inelastic x-ray scattering measurements of the acoustic phonons of URu2Si2. At all temperatures, the longitudinal acoustic phonon linewidths are anomalously broad at small wave vectors revealing a previously unknown anharmonicity. The phonon modes do not change significantly upon cooling into the hidden order phase. In addition, our data suggest that the increase in thermal conductivity in the hidden order phase cannot be driven by a change in phonon dispersions or lifetimes. Hence, the phonon contribution to the thermal conductivity is likely much less significant compared to that of the magnetic excitations in the lowmore » temperature phase.« less

  7. Picosecond x-ray strain rosette reveals direct laser excitation of coherent transverse acoustic phonons

    PubMed Central

    Lee, Sooheyong; Williams, G. Jackson; Campana, Maria I.; Walko, Donald A.; Landahl, Eric C.

    2016-01-01

    Using a strain-rosette, we demonstrate the existence of transverse strain using time-resolved x-ray diffraction from multiple Bragg reflections in laser-excited bulk gallium arsenide. We find that anisotropic strain is responsible for a considerable fraction of the total lattice motion at early times before thermal equilibrium is achieved. Our measurements are described by a new model where the Poisson ratio drives transverse motion, resulting in the creation of shear waves without the need for an indirect process such as mode conversion at an interface. Using the same excitation geometry with the narrow-gap semiconductor indium antimonide, we detected coherent transverse acoustic oscillations at frequencies of several GHz. PMID:26751616

  8. Picosecond x-ray strain rosette reveals direct laser excitation of coherent transverse acoustic phonons

    SciTech Connect

    Lee, Sooheyong; Williams, G. Jackson; Campana, Maria I.; Walko, Donald A.; Landahl, Eric C.

    2016-01-11

    Using a strain-rosette, we demonstrate the existence of transverse strain using time-resolved x-ray diffraction from multiple Bragg reflections in laser-excited bulk gallium arsenide. We find that anisotropic strain is responsible for a considerable fraction of the total lattice motion at early times before thermal equilibrium is achieved. Our measurements are described by a new model where the Poisson ratio drives transverse motion, resulting in the creation of shear waves without the need for an indirect process such as mode conversion at an interface. Finally, using the same excitation geometry with the narrow-gap semiconductor indium antimonide, we detected coherent transverse acoustic oscillations at frequencies of several GHz.

  9. Acoustic Typology of Vowel Inventories and Dispersion Theory: Insights from a Large Cross-Linguistic Corpus

    ERIC Educational Resources Information Center

    Becker-Kristal, Roy

    2010-01-01

    This dissertation examines the relationship between the structural, phonemic properties of vowel inventories and their acoustic phonetic realization, with particular focus on the adequacy of Dispersion Theory, which maintains that inventories are structured so as to maximize perceptual contrast between their component vowels. In order to assess…

  10. Nonlinear Acoustics in a Dispersive Continuum: Random Waves, Radiation Pressure, and Quantum Noise.

    DTIC Science & Technology

    1983-03-01

    Karpman , Nonlinear Waves in Dispersive Media, Pergamon Press, New York, 1975, p. 76. 26. R. Beyers, Nonlinear Acoustics, U.S. Government Printing...20301 U. S. Army Research nffice 2 copies Box 12211 Research Triangle Park tlorth Carolina 27709 Defense Technical Information Center 12 copies Cameron

  11. Pre-transitional evolution of central peaks and transverse acoustic phonon branch in single crystal lead zirconate titanate with Ti concentration 0.7%

    NASA Astrophysics Data System (ADS)

    Andronikova, D. A.; Bronwald, I. A.; Burkovsky, R. G.; Leontiev, I. N.; Leontiev, N. G.; Bosak, A. A.; Filimonov, A. V.; Vakhrushev, S. B.

    2016-11-01

    Inelastic X-ray scattering measurements have been done to study the lattice dynamics in lead zirconate titanate solid solution with 0.7% of PbTiO3. The temperature evolution of central peak and low-energy transverse phonon branches has been traced. Temperature dependent in-plane transverse polarized acoustic phonon branch in <1 1 0> direction has been revealed. The central peaks of two types have been found. The central peak at small wave vectors can be attributed to the relaxational-type soft ferroelectric mode, while the latter at Q = (1.5 -0.5 0) could be linked to the formation of M-superstructure in the intermediate ferroelectric phase.

  12. Phonon properties of americium phosphide

    NASA Astrophysics Data System (ADS)

    Arya, B. S.; Aynyas, Mahendra; Sanyal, S. P.

    2016-05-01

    Phonon properties of AmP have been studied by using breathing shell models (BSM) which includes breathing motion of electrons of the Am atoms due to f-d hybridization. The phonon dispersion curves, specific heat calculated from present model. The calculated phonon dispersion curves of AmP are presented follow the same trend as observed in uranium phosphide. We discuss the significance of this approach in predicting the phonon dispersion curves of these compounds and examine the role of electron-phonon interaction.

  13. Phonon Spectrum Engineering in Rolled-up Micro- and Nano-Architectures

    SciTech Connect

    Fomin, Vladimir M.; Balandin, Alexander A.

    2015-10-10

    We report on a possibility of efficient engineering of the acoustic phonon energy spectrum in multishell tubular structures produced by a novel high-tech method of self-organization of micro- and nano-architectures. The strain-driven roll-up procedure paved the way for novel classes of metamaterials such as single semiconductor radial micro- and nano-crystals and multi-layer spiral micro- and nano-superlattices. The acoustic phonon dispersion is determined by solving the equations of elastodynamics for InAs and GaAs material systems. It is shown that the number of shells is an important control parameter of the phonon dispersion together with the structure dimensions and acoustic impedance mismatch between the superlattice layers. The obtained results suggest that rolled up nano-architectures are promising for thermoelectric applications owing to a possibility of significant reduction of the thermal conductivity without degradation of the electronic transport.

  14. Phonon Spectrum Engineering in Rolled-up Micro- and Nano-Architectures

    DOE PAGES

    Fomin, Vladimir M.; Balandin, Alexander A.

    2015-10-10

    We report on a possibility of efficient engineering of the acoustic phonon energy spectrum in multishell tubular structures produced by a novel high-tech method of self-organization of micro- and nano-architectures. The strain-driven roll-up procedure paved the way for novel classes of metamaterials such as single semiconductor radial micro- and nano-crystals and multi-layer spiral micro- and nano-superlattices. The acoustic phonon dispersion is determined by solving the equations of elastodynamics for InAs and GaAs material systems. It is shown that the number of shells is an important control parameter of the phonon dispersion together with the structure dimensions and acoustic impedance mismatchmore » between the superlattice layers. The obtained results suggest that rolled up nano-architectures are promising for thermoelectric applications owing to a possibility of significant reduction of the thermal conductivity without degradation of the electronic transport.« less

  15. Broadband evolution of phononic-crystal-waveguide eigenstates in real- and k-spaces.

    PubMed

    Otsuka, P H; Nanri, K; Matsuda, O; Tomoda, M; Profunser, D M; Veres, I A; Danworaphong, S; Khelif, A; Benchabane, S; Laude, V; Wright, O B

    2013-11-27

    Control of sound in phononic band-gap structures promises novel control and guiding mechanisms. Designs in photonic systems were quickly matched in phononics, and rows of defects in phononic crystals were shown to guide sound waves effectively. The vast majority of work in such phononic guiding has been in the frequency domain, because of the importance of the phononic dispersion relation in governing acoustic confinement in waveguides. However, frequency-domain studies miss vital information concerning the phase of the acoustic field and eigenstate coupling. Using a wide range of wavevectors k, we implement an ultrafast technique to probe the wave field evolution in straight and L-shaped phononic crystal surface-phonon waveguides in real- and k-space in two spatial dimensions, thus revealing the eigenstate-energy redistribution processes and the coupling between different frequency-degenerate eigenstates. Such use of k-t space is a first in acoustics, and should have other interesting applications such as acoustic-metamaterial characterization.

  16. Study on the properties of vacancies and phonon dispersions by the improved ones of the modified analytic embedded atom method potentials for Al, Ni, and Ir

    NASA Astrophysics Data System (ADS)

    Jin, Hak-Son; Pak, Jae-Yon; Jong, Yon-Song

    2017-04-01

    The properties of the mono- and bi-vacancies and the phonon dispersions are calculated by adopting the improved ones of the modified analytical embedded atom method potentials for facet-centered cubic metals Al, Ni, and Ir. The results mainly agree with the experimental data and the other calculation results. Therefore, the improved potentials are effective in the study on the physical properties of the metals.

  17. Electron-phonon coupling and thermal transport in thermoelectric compound Mo3Sb7-xTex

    NASA Astrophysics Data System (ADS)

    Bansal, Dipanshu; Li, Chen; Said, Ayman; Abernathy, Douglas; Yan, Jiaqiang; Delaire, Olivier

    Complex interactions between solid-state excitations, such as phonon-phonon, phonon-electron, and phonon-magnon couplings are often responsible for unusual material properties. In this presentation, we report on our investigations of phonon propagation and thermal transport in thermoelectric Mo3Sb7-xTex. We have performed extensive inelastic neutron and x-ray scattering measurements of phonons in Mo3Sb7-xTex, mapping the phonon dispersions and density of states, as function of temperature and composition. Our first-principles density functional theory simulations, coupled with experimental measurements, reveal the importance of electron-phonon coupling, which dominates the scattering rates over alloy disorder scattering. Doping with Te shifts the Fermi surface near the top of the valence band, suppressing screening and causing phonons to stiffen markedly. Our measurements of acoustic dispersions and linewidths, coupled with DFT simulations and models of phonon scattering enable us to quantify the impact of the electron-phonon coupling on the thermal conductivity.

  18. Acoustic phonon-limited resistivity of spin-orbit coupled two-dimensional electron gas: the deformation potential and piezoelectric scattering.

    PubMed

    Biswas, Tutul; Ghosh, Tarun Kanti

    2013-01-23

    We study the interaction between electron and acoustic phonons in a Rashba spin-orbit coupled two-dimensional electron gas using Boltzmann transport theory. Both the deformation potential and piezoelectric scattering mechanisms are considered in the Bloch-Grüneisen (BG) regime as well as in the equipartition (EP) regime. The effect of the Rashba spin-orbit interaction on the temperature dependence of the resistivity in the BG and EP regimes is discussed. We find that the effective exponent of the temperature dependence of the resistivity in the BG regime decreases due to spin-orbit coupling.

  19. First-principles prediction of phononic thermal conductivity of silicene: A comparison with graphene

    SciTech Connect

    Gu, Xiaokun; Yang, Ronggui

    2015-01-14

    There has been great interest in two-dimensional materials, beyond graphene, for both fundamental sciences and technological applications. Silicene, a silicon counterpart of graphene, has been shown to possess some better electronic properties than graphene. However, its thermal transport properties have not been fully studied. In this paper, we apply the first-principles-based phonon Boltzmann transport equation to investigate the thermal conductivity of silicene as well as the phonon scattering mechanisms. Although both graphene and silicene are two-dimensional crystals with similar crystal structure, we find that phonon transport in silicene is quite different from that in graphene. The thermal conductivity of silicene shows a logarithmic increase with respect to the sample size due to the small scattering rates of acoustic in-plane phonon modes, while that of graphene is finite. Detailed analysis of phonon scattering channels shows that the linear dispersion of the acoustic out-of-plane (ZA) phonon modes, which is induced by the buckled structure, makes the long-wavelength longitudinal acoustic phonon modes in silicene not as efficiently scattered as that in graphene. Compared with graphene, where most of the heat is carried by the acoustic out-of-plane (ZA) phonon modes, the ZA phonon modes in silicene only have ∼10% contribution to the total thermal conductivity, which can also be attributed to the buckled structure. This systematic comparison of phonon transport and thermal conductivity of silicene and graphene using the first-principle-based calculations shed some light on other two-dimensional materials, such as two-dimensional transition metal dichalcogenides.

  20. Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2

    SciTech Connect

    Gardner, D. R.; Bonnoit, C. J.; Chisnell, R.; Said, A. H.; Leu, B. M.; Williams, Travis J.; Luke, G. M.; Lee, Y. S.

    2016-02-11

    In this paper, we study high-resolution inelastic x-ray scattering measurements of the acoustic phonons of URu2Si2. At all temperatures, the longitudinal acoustic phonon linewidths are anomalously broad at small wave vectors revealing a previously unknown anharmonicity. The phonon modes do not change significantly upon cooling into the hidden order phase. In addition, our data suggest that the increase in thermal conductivity in the hidden order phase cannot be driven by a change in phonon dispersions or lifetimes. Hence, the phonon contribution to the thermal conductivity is likely much less significant compared to that of the magnetic excitations in the low temperature phase.

  1. Nonlinear phononics using atomically thin membranes

    NASA Astrophysics Data System (ADS)

    Midtvedt, Daniel; Isacsson, Andreas; Croy, Alexander

    2014-09-01

    Phononic crystals and acoustic metamaterials are used to tailor phonon and sound propagation properties by utilizing artificial, periodic structures. Analogous to photonic crystals, phononic band gaps can be created, which influence wave propagation and, more generally, allow engineering of the acoustic properties of a system. Beyond that, nonlinear phenomena in periodic structures have been extensively studied in photonic crystals and atomic Bose-Einstein condensates in optical lattices. However, creating nonlinear phononic crystals or nonlinear acoustic metamaterials remains challenging and only few examples have been demonstrated. Here, we show that atomically thin and periodically pinned membranes support coupled localized modes with nonlinear dynamics. The proposed system provides a platform for investigating nonlinear phononics.

  2. Measurements of Finite Dust Temperature Effects in the Dispersion Relation of the Dust Acoustic Wave

    NASA Astrophysics Data System (ADS)

    Snipes, Erica; Williams, Jeremiah

    2009-04-01

    A dusty plasma is a four-component system composed of ions, electrons, neutral particles and charged microparticles. The presence of these charged microparticles gives rise to new plasma wave modes, including the dust acoustic wave. Recent measurements [1, 2] of the dispersion relationship for the dust acoustic wave in a glow discharge have shown that finite temperature effects are observed at higher values of neutral pressure. Other work [3] has shown that these effects are not observed at lower values of neutral pressure. We present the results of ongoing work examining finite temperature effects in the dispersion relation as a function of neutral pressure. [4pt] [1] E. Thomas, Jr., R. Fisher, and R. L. Merlino, Phys. Plasmas 14, 123701 (2007). [0pt] [2] J. D. Williams, E. Thomas Jr., and L. Marcus, Phys. Plasmas 15, 043704 (2008). [0pt] [3] T. Trottenberg, D. Block, and A. Piel, Phys. Plasmas 13, 042105 (2006).

  3. Acoustic emission localization in plates with dispersion and reverberations using sparse PZT sensors in passive mode

    NASA Astrophysics Data System (ADS)

    Perelli, Alessandro; De Marchi, Luca; Marzani, Alessandro; Speciale, Nicolò

    2012-02-01

    A strategy for the localization of acoustic emissions (AE) in plates with dispersion and reverberation is proposed. The procedure exploits signals received in passive mode by sparse conventional piezoelectric transducers and a three-step processing framework. The first step consists in a signal dispersion compensation procedure, which is achieved by means of the warped frequency transform. The second step concerns the estimation of the differences in arrival time (TDOA) of the acoustic emission at the sensors. Complexities related to reflections and plate resonances are overcome via a wavelet decomposition of cross-correlating signals where the mother function is designed by a synthetic warped cross-signal. The magnitude of the wavelet coefficients in the warped distance-frequency domain, in fact, precisely reveals the TDOA of an acoustic emission at two sensors. Finally, in the last step the TDOA data are exploited to locate the acoustic emission source through hyperbolic positioning. The proposed procedure is tested with a passive network of three/four piezo-sensors located symmetrically and asymmetrically with respect to the plate edges. The experimentally estimated AE locations are close to those theoretically predicted by the Cramèr-Rao lower bound.

  4. Resonance damping of the terahertz-frequency transverse acoustic phonon in the relaxor ferroelectric KT a1 -xN bxO3

    NASA Astrophysics Data System (ADS)

    Toulouse, J.; Iolin, E.; Hennion, B.; Petitgrand, D.; Erwin, R.

    2016-12-01

    The damping (Γ a ) of the transverse acoustic (TA) phonon in single crystals of the relaxor KT a1 -xN bxO3 with x =0.15 -0.17 was studied by means of high resolution inelastic cold neutron scattering near the (200) Brillouin Zone (BZ) point where diffuse scattering is absent, although it is present near (110). In a wide range of temperatures centered on the phase transition, T =195 K ÷108 K , the TA phonon width (damping) exhibits a step increase around momentum q =0.07 , goes through a shallow maximum at q =0.09 -0.12 , and remains high above and up to the highest momentum studied of q =0.16 . These experimental results are explained in terms of a resonant interaction between the TA phonon and the collective or correlated reorientation through tunneling of the off-center N b+5 ions. The observed TA damping is successfully reproduced in a simple model that includes an interaction between the TA phonon and a dispersionless localized mode (LM) with frequency ωL and damping ΓL(ΓL<ωL) , itself coupled to the transverse optic (TO) mode. Maximum damping of the TA phonon occurs when its frequency is ωa≈ωL . The values of ωL and ΓL are moderately dependent on temperature, but the oscillator strength, M2, of the resonant damping exhibits a strong maximum in the range T ˜120 K ÷150 K in which neutron diffuse scattering near the (110) BZ point is also maximum and the dielectric susceptibility exhibits the relaxor behavior. The maximum value of M appears to be due to the increasing number of polar nanodomains. In support of the proposed model, the observed value of ωL≈0.7 THz is found to be similar to the estimate previously obtained by Girshberg and Yacoby [J. Phys.: Condens. Matter 24, 015901 (2012)], 10.1088/0953-8984/24/1/015901. Alternatively, the TA phonon damping can be successfully fitted in the framework of an empirical Havriliak-Negami (HN) relaxation model that includes a strong resonancelike transient contribution.

  5. Size-Dependent Coherent-Phonon Plasmon Modulation and Deformation Characterization in Gold Bipyramids and Nanojavelins

    SciTech Connect

    Kirschner, Matthew S.; Lethiec, Clotilde M.; Lin, Xiao-Min; Schatz, George C.; Chen, Lin X.; Schaller, Richard D.

    2016-05-18

    Localized surface plasmon resonances (LSPRs) arising from metallic nanoparticles offer an array of prospective applications that range from chemical sensing to biotherapies. Bipyramidal particles exhibit particularly narrow ensemble LSPR resonances that reflect small dispersity of size and shape but until recently were only synthetically accessible over a limited range of sizes with corresponding aspect ratios. Narrow size dispersion offers the opportunity to examine ensemble dynamical phenomena such as coherent phonons that induce periodic oscillations of the LSPR energy. Here, we characterize transient optical behavior of a large range of gold bipyramid sizes, as well as higher aspect ratio nanojavelin ensembles with specific attention to the lowest-order acoustic phonon mode of these nanoparticles. We report coherent phonon-driven oscillations of the LSPR position for particles with resonances spanning 670 to 1330 nm. Nanojavelins were shown to behave similarly to bipyramids but offer the prospect of separate control over LSPR energy and coherent phonon oscillation period. We develop a new methodology for quantitatively measuring mechanical expansion caused by photogenerated coherent phonons. Using this method, we find an elongation of approximately 1% per photon absorbed per unit cell and that particle expansion along the lowest frequency acoustic phonon mode is linearly proportional to excitation fluence for the fluence range studied. These characterizations provide insight regarding means to manipulate phonon period and transient mechanical deformation.

  6. Cavity-type hypersonic phononic crystals

    NASA Astrophysics Data System (ADS)

    Sato, A.; Pennec, Y.; Yanagishita, T.; Masuda, H.; Knoll, W.; Djafari-Rouhani, B.; Fytas, G.

    2012-11-01

    We report on the engineering of the phonon dispersion diagram in monodomain anodic porous alumina (APA) films through the porosity and physical state of the material residing in the nanopores. Lattice symmetry and inclusion materials are theoretically identified to be the main factors which control the hypersonic acoustic wave propagation. This involves the interaction between the longitudinal and the transverse modes in the effective medium and a flat band characteristic of the material residing in the cavities. Air and filled nanopores, therefore, display markedly different dispersion relations and the inclusion materials lead to a locally resonant structural behavior uniquely determining their properties under confinement. APA films emerge as a new platform to investigate the rich acoustic phenomena of structured composite matter.

  7. Extremely Efficient Liquid Exfoliation and Dispersion of Layered Materials by Unusual Acoustic Cavitation

    PubMed Central

    Han, Joong Tark; Jang, Jeong In; Kim, Haena; Hwang, Jun Yeon; Yoo, Hyung Keun; Woo, Jong Seok; Choi, Sua; Kim, Ho Young; Jeong, Hee Jin; Jeong, Seung Yol; Baeg, Kang-Jun; Cho, Kilwon; Lee, Geon-Woong

    2014-01-01

    Layered materials must be exfoliated and dispersed in solvents for diverse applications. Usually, highly energetic probe sonication may be considered to be an unfavourable method for the less defective exfoliation and dispersion of layered materials. Here we show that judicious use of ultrasonic cavitation can produce exfoliated transition metal dichalcogenide nanosheets extraordinarily dispersed in non-toxic solvent by minimising the sonolysis of solvent molecules. Our method can also lead to produce less defective, large graphene oxide nanosheets from graphite oxide in a short time (within 10 min), which show high electrical conductivity (>20,000 S m−1) of the printed film. This was achieved by adjusting the ultrasonic probe depth to the liquid surface to generate less energetic cavitation (delivered power ~6 W), while maintaining sufficient acoustic shearing (0.73 m s−1) and generating additional microbubbling by aeration at the liquid surface. PMID:24875584

  8. Phase-based dispersion analysis for acoustic array borehole logging data.

    PubMed

    Assous, Said; Elkington, Peter; Linnett, Laurie

    2014-04-01

    A phase-based dispersion analysis method for velocity (slowness) extraction from guided waves recorded by an acoustic borehole logging tool in a geological formation is presented. The technique consists of acquiring waveforms from an array of receivers distributed along the tool and constructing the dispersion characteristic by processing in the frequency domain and exploiting phase information to measure the travel time for each frequency component. The approach is nonparametric and completely data-driven and provides high resolution estimates that do not rely on velocity guesses or assumptions regarding the type of modes. Results are free of the aliases and spurious modes which are characteristic of some prior approaches. Examples of dispersion estimation curves are presented using synthesized flexural waves and field data from wireline dipole sonic tools; results are compared with those from the weighted spectral semblance (WSS) and amplitude and phase slowness estimation (APES) methods to demonstrate the effectiveness and utility of the proposed method.

  9. Systematic investigation of effects of exciton–acoustic-phonon scattering on photoluminescence rise times of free excitons in GaAs/Al{sub 0.3}Ga{sub 0.7}As single quantum wells

    SciTech Connect

    Nakayama, Masaaki Ohno, Tatsuya; Furukawa, Yoshiaki

    2015-04-07

    We have systematically investigated the photoluminescence (PL) dynamics of free excitons in GaAs/Al{sub 0.3}Ga{sub 0.7}As single quantum wells, focusing on the energy relaxation process due to exciton–acoustic-phonon scattering under non-resonant and weak excitation conditions as a function of GaAs-layer thickness from 3.6 to 12.0 nm and temperature from 30 to 50 K. The free exciton characteristics were confirmed by observation that the PL decay time has a linear dependence with temperature. We found that the free exciton PL rise rate, which is the reciprocal of the rise time, is inversely linear with the GaAs-layer thickness and linear with temperature. This is consistent with a reported theoretical study of the exciton–acoustic-phonon scattering rate in the energy relaxation process in quantum wells. Consequently, it is conclusively verified that the PL rise rate is dominated by the exciton–acoustic-phonon scattering rate. In addition, from quantitative analysis of the GaAs-layer thickness and temperature dependences, we suggest that the PL rise rate reflects the number of exciton–acoustic-phonon scattering events.

  10. Dispersion, dissipation and refraction of shock waves in acoustically treated turbofan inlets

    NASA Astrophysics Data System (ADS)

    Prasad, Dilip; Li, Ding; A. Topol, David

    2015-09-01

    This paper describes a numerical investigation of the effects of the inlet duct liner on the acoustics of a high-bypass ratio turbofan rotor operating at supersonic tip relative flow conditions. The near field of the blade row is then composed of periodic shocks that evolve spatially both because of the varying mean flow and because of the presence of acoustic treatment. The evolution of this shock system is studied using a Computational Fluid Dynamics-based method incorporating a wall impedance boundary condition. The configuration examined is representative of a fan operating near the takeoff condition. The behavior of the acoustic power and the associated waveforms reveal that significant dispersion occurs to the extent that there are no shocks in the perturbation field leaving the entrance plane of the duct. The effect of wave refraction due to the high degree of shear in the mean flow near the entrance plane of the inlet is examined, and numerical experiments are conducted to show that the incorporation of liners in this region can be highly beneficial. The implications of these results for the design of aircraft engine acoustic liners are discussed.

  11. Influence of Acoustic and Electromagnetic Actions on the Properties of Aqueous Nanoparticle Dispersions Used as Tempering Liquids for Dental Cement

    NASA Astrophysics Data System (ADS)

    Azharonok, V. V.; Belous, N. Kh.; Rodtsevich, S. P.; Goncharik, S. V.; Chubrik, N. N.; Koshevar, V. D.; Lopat‧ko, K. G.; Aftandilyants, E. G.; Veklich, A. N.; Boretskii, V. F.; Orlovich, A. I.

    2016-05-01

    The authors have studied the physicochemical properties of aqueous dispersions containing carbon, silver, and iron nanoparticles which were produced by elastic-spark synthesis under the conditions of subaqueous spark discharge, and also the influence of preliminary acoustic and high-frequency electromagnetic action on them and the change in the functional indices of the glass-ionomer cement tempered by these dispersions.

  12. Estimating sub-surface dispersed oil concentration using acoustic backscatter response.

    PubMed

    Fuller, Christopher B; Bonner, James S; Islam, Mohammad S; Page, Cheryl; Ojo, Temitope; Kirkey, William

    2013-05-15

    The recent Deepwater Horizon disaster resulted in a dispersed oil plume at an approximate depth of 1000 m. Several methods were used to characterize this plume with respect to concentration and spatial extent including surface supported sampling and autonomous underwater vehicles with in situ instrument payloads. Additionally, echo sounders were used to track the plume location, demonstrating the potential for remote detection using acoustic backscatter (ABS). This study evaluated use of an Acoustic Doppler Current Profiler (ADCP) to quantitatively detect oil-droplet suspensions from the ABS response in a controlled laboratory setting. Results from this study showed log-linear ABS responses to oil-droplet volume concentration. However, the inability to reproduce ABS response factors suggests the difficultly in developing meaningful calibration factors for quantitative field analysis. Evaluation of theoretical ABS intensity derived from the particle size distribution provided insight regarding method sensitivity in the presence of interfering ambient particles.

  13. Algorithmic Extensions of Low-Dispersion Scheme and Modeling Effects for Acoustic Wave Simulation. Revised

    NASA Technical Reports Server (NTRS)

    Kaushik, Dinesh K.; Baysal, Oktay

    1997-01-01

    Accurate computation of acoustic wave propagation may be more efficiently performed when their dispersion relations are considered. Consequently, computational algorithms which attempt to preserve these relations have been gaining popularity in recent years. In the present paper, the extensions to one such scheme are discussed. By solving the linearized, 2-D Euler and Navier-Stokes equations with such a method for the acoustic wave propagation, several issues were investigated. Among them were higher-order accuracy, choice of boundary conditions and differencing stencils, effects of viscosity, low-storage time integration, generalized curvilinear coordinates, periodic series, their reflections and interference patterns from a flat wall and scattering from a circular cylinder. The results were found to be promising en route to the aeroacoustic simulations of realistic engineering problems.

  14. Anharmonic free energies and phonon dispersions from the stochastic self-consistent harmonic approximation: Application to platinum and palladium hydrides

    NASA Astrophysics Data System (ADS)

    Errea, Ion; Calandra, Matteo; Mauri, Francesco

    2014-02-01

    Harmonic calculations based on density-functional theory are generally the method of choice for the description of phonon spectra of metals and insulators. The inclusion of anharmonic effects is, however, delicate as it relies on perturbation theory requiring a considerable amount of computer time, fast increasing with the cell size. Furthermore, perturbation theory breaks down when the harmonic solution is dynamically unstable or the anharmonic correction of the phonon energies is larger than the harmonic frequencies themselves. We present here a stochastic implementation of the self-consistent harmonic approximation valid to treat anharmonicity at any temperature in the nonperturbative regime. The method is based on the minimization of the free energy with respect to a trial density matrix described by an arbitrary harmonic Hamiltonian. The minimization is performed with respect to all the free parameters in the trial harmonic Hamiltonian, namely, equilibrium positions, phonon frequencies, and polarization vectors. The gradient of the free energy is calculated following a stochastic procedure. The method can be used to calculate thermodynamic properties, dynamical properties, and even anharmonic corrections to the Eliashberg function of the electron-phonon coupling. The scaling with the system size is greatly improved with respect to perturbation theory. The validity of the method is demonstrated in the strongly anharmonic palladium and platinum hydrides. In both cases, we predict a strong anharmonic correction to the harmonic phonon spectra, far beyond the perturbative limit. In palladium hydrides, we calculate thermodynamic properties beyond the quasiharmonic approximation, while in PtH, we demonstrate that the high superconducting critical temperatures at 100 GPa predicted in previous calculations based on the harmonic approximation are strongly suppressed when anharmonic effects are included.

  15. Acoustic phonon assisted free-carrier optical absorption in an n-type monolayer MoS{sub 2} and other transition-metal dichalcogenides

    SciTech Connect

    Bhargavi, K. S.; Patil, Sukanya; Kubakaddi, S. S.

    2015-07-28

    The theory of free-carrier absorption (FCA) is given for monolayers of transition-metal dichalcogenides, particularly for molybdenum disulphide (MoS{sub 2}), when carriers are scattered by phonons. Explicit expressions for the absorption coefficient α are obtained and discussed for acoustic phonon scattering via screened deformation potential and piezoelectric coupling taking polarization of the radiation in the plane of the layer. It is found that α monotonously decreases with the increasing photon frequency Ω, increases with the increasing temperature T, and linearly depends on two-dimensional electron concentration n{sub s}. Effect of screening, which is ignored in all the earlier FCA studies, is found to reduce α significantly, attributing to the larger effective mass of the electrons. Results are also obtained in the classical and quantum limit giving the power laws α ∼ Ω{sup −2} and T. Comparison of the results is made with those in bulk semiconductors and semiconductor quantum wells.

  16. Isotope scattering and phonon thermal conductivity in light atom compounds: LiH and LiF

    NASA Astrophysics Data System (ADS)

    Lindsay, L.

    2016-11-01

    Engineered isotope variation is a pathway toward modulating lattice thermal conductivity (κ) of a material through changes in phonon-isotope scattering. The effects of isotope variation on intrinsic thermal resistance is little explored, as varying isotopes have relatively small differences in mass and thus do not affect bulk phonon dispersions. However, for light elements, isotope mass variation can be relatively large (e.g., hydrogen and deuterium). Using a first principles Peierls-Boltzmann transport equation approach, the effects of isotope variance on lattice thermal transport in ultra-low-mass compound materials LiH and LiF are characterized. The isotope mass variance modifies the intrinsic thermal resistance via modulation of acoustic and optic phonon frequencies, while phonon-isotope scattering from mass disorder plays only a minor role. This leads to some unusual cases where κ values of isotopically pure systems (6LiH ,7L i2H , and 6LiF ) are lower than the values from their counterparts with naturally occurring isotopes and phonon-isotope scattering. However, these κ differences are relatively small. The effects of temperature-driven lattice expansion on phonon dispersions and calculated κ are also discussed. This paper provides insight into lattice thermal conductivity modulation with mass variation and the interplay of intrinsic phonon-phonon and phonon-isotope scattering in interesting light atom systems.

  17. Isotope scattering and phonon thermal conductivity in light atom compounds: LiH and LiF

    DOE PAGES

    Lindsay, Lucas R.

    2016-11-08

    Engineered isotope variation is a pathway toward modulating lattice thermal conductivity (κ) of a material through changes in phonon-isotope scattering. The effects of isotope variation on intrinsic thermal resistance is little explored, as varying isotopes have relatively small differences in mass and thus do not affect bulk phonon dispersions. However, for light elements isotope mass variation can be relatively large (e.g., hydrogen and deuterium). Using a first principles Peierls-Boltzmann transport equation approach the effects of isotope variance on lattice thermal transport in ultra-low-mass compound materials LiH and LiF are characterized. The isotope mass variance modifies the intrinsic thermal resistance viamore » modulation of acoustic and optic phonon frequencies, while phonon-isotope scattering from mass disorder plays only a minor role. This leads to some unusual cases where values of isotopically pure systems (6LiH, 7Li2H and 6LiF) are lower than the values from their counterparts with naturally occurring isotopes and phonon-isotope scattering. However, these differences are relatively small. The effects of temperature-driven lattice expansion on phonon dispersions and calculated κ are also discussed. This work provides insight into lattice thermal conductivity modulation with mass variation and the interplay of intrinsic phonon-phonon and phonon-isotope scattering in interesting light atom systems.« less

  18. Isotope scattering and phonon thermal conductivity in light atom compounds: LiH and LiF

    SciTech Connect

    Lindsay, Lucas R.

    2016-11-08

    Engineered isotope variation is a pathway toward modulating lattice thermal conductivity (κ) of a material through changes in phonon-isotope scattering. The effects of isotope variation on intrinsic thermal resistance is little explored, as varying isotopes have relatively small differences in mass and thus do not affect bulk phonon dispersions. However, for light elements isotope mass variation can be relatively large (e.g., hydrogen and deuterium). Using a first principles Peierls-Boltzmann transport equation approach the effects of isotope variance on lattice thermal transport in ultra-low-mass compound materials LiH and LiF are characterized. The isotope mass variance modifies the intrinsic thermal resistance via modulation of acoustic and optic phonon frequencies, while phonon-isotope scattering from mass disorder plays only a minor role. This leads to some unusual cases where values of isotopically pure systems (6LiH, 7Li2H and 6LiF) are lower than the values from their counterparts with naturally occurring isotopes and phonon-isotope scattering. However, these differences are relatively small. The effects of temperature-driven lattice expansion on phonon dispersions and calculated κ are also discussed. This work provides insight into lattice thermal conductivity modulation with mass variation and the interplay of intrinsic phonon-phonon and phonon-isotope scattering in interesting light atom systems.

  19. Problems in Nonlinear Acoustics: Parametric Receiving Arrays, Focused Finite Amplitude Sound, and Dispersive Nonlinear Interactions.

    DTIC Science & Technology

    1986-04-30

    TenCate , who is supported by ONR Contract NOOO I 4-84-K-0574, in the completion of work on pure tones that interact in higher order modes of a...rectangular duct.26 Through collaboration with TenCate , Lind has acquired experience with the same experimental apparatus that he will use beginning I June...34 J. Acoust. Soc. " .. Am. 65.1127-1133(1979). 36. J. A TenCate and K F. Hamilton, "Dispersive nonlinear wave interactions in a rectangular duct," In

  20. ``Forbidden'' phonon in the iron chalcogenide series

    NASA Astrophysics Data System (ADS)

    Fobes, David M.; Zaliznyak, Igor A.; Xu, Zhijun; Gu, Genda; Tranquada, John M.

    2015-03-01

    Recently, we uncovered evidence for the formation of a bond-order wave (BOW) leading to ferro-orbital order at low temperature, acting to stabilize the bicollinear AFM order, in the iron-rich parent compound, Fe1+yTe. Investigating the inelastic spectra centered near (100) in Fe1+yTe, a signature peak for the BOW formation in the monoclinic phase, we observed an acoustic phonon dispersion in both tetragonal and monoclinic phases. While a structural Bragg peak accompanies the mode in the monoclinic phase, in the tetragonal phase Bragg scattering at this Q is forbidden by symmetry, and we observed no elastic peak. This phonon mode was also observed in superconducting FeTe0.6Se0.4, where structural and magnetic transitions are suppressed. LDA frozen phonon calculations suggested that this mode could result from a spin imbalance between neighboring Fe atoms, but polarized neutron measurements revealed no additional magnetic scattering. We propose that this ``forbidden'' phonon mode may originate from dynamically broken symmetry, perhaps related to the strong dynamic spin correlations in these materials. Work at BNL was supported by BES, US DOE, under Contract No. DE-AC02-98CH10886. Research at ORNL's HFIR and SNS sponsored by Scientific User Facilities Division, BES, US DOE. We acknowledge the support of NIST, in providing neutron research facilities.

  1. Geometric tuning of thermal conductivity in three-dimensional anisotropic phononic crystals.

    PubMed

    Wei, Zhiyong; Wehmeyer, Geoff; Dames, Chris; Chen, Yunfei

    2016-10-07

    Molecular dynamics simulations are performed to investigate the thermal transport properties of a three-dimensional (3D) anisotropic phononic crystal consisting of silicon nanowires and films. The calculation shows that the in-plane thermal conductivity is negatively correlated with the out-of-plane thermal conductivity upon making geometric changes, whether varying the nanowire diameter or the film thickness. This enables the anisotropy ratio of thermal conductivity to be tailored over a wide range, in some cases by more than a factor of 20. Similar trends in thermal conductivity are also observed from an independent phonon ray tracing simulation considering only diffuse boundary scattering effects, though the range of anisotropy ratios is smaller than that obtained in MD simulation. By analyzing the phonon dispersion relation with varied geometric parameters, it is found that increasing the nanowire diameter increases the out-of-plane acoustic phonon group velocities, but reduces the in-plane longitudinal and fast transverse acoustic phonon group velocities. The calculated phonon irradiation further verified the negative correlation between the in-plane and the out-of-plane thermal conductivity. The proposed 3D phononic crystal may find potential application in thermoelectrics, energy storage, catalysis and sensing applications owing to its widely tailorable thermal conductivity.

  2. Complex dispersion relation of surface acoustic waves at a lossy metasurface

    NASA Astrophysics Data System (ADS)

    Schwan, Logan; Geslain, Alan; Romero-García, Vicente; Groby, Jean-Philippe

    2017-01-01

    The complex dispersion relation of surface acoustic waves (SAWs) at a lossy resonant metasurface is theoretically and experimentally reported. The metasurface consists of the periodic arrangement of borehole resonators in a rigid substrate. The theoretical model relies on a boundary layer approach that provides the effective metasurface admittance governing the complex dispersion relation in the presence of viscous and thermal losses. The model is experimentally validated by measurements in the semi-anechoic chamber. The complex SAW dispersion relation is experimentally retrieved from the analysis of the spatial Laplace transform of the pressure scanned along a line at the metasurface. The geometrical spreading of the energy from the speaker is accounted for, and both the real and imaginary parts of the SAW wavenumber are obtained. The results show that the strong reduction of the SAW group velocity occurs jointly with a drastic attenuation of the wave, leading to the confinement of the field close to the source and preventing the efficient propagation of such slow-sound surface modes. The method opens perspectives to theoretically predict and experimentally characterize both the dispersion and the attenuation of surface waves at structured surfaces.

  3. Doppler acoustic sounding: observational inputs to pollutant-dispersion models. Final report

    SciTech Connect

    MacCready, P.; Worden, J.

    1982-01-01

    To accurately model the dilution of pollutants, as in the form of plumes from large power plants, actual observations of atmospheric characteristics aloft are needed. The goal of this program was to find out whether a portable, multi-beam, monostatic Doppler acoustic system (DAS) can provide the measurements of conditions aloft that are required as inputs to dispersion models suitable for routine applications. Evaluation of what the Doppler system can measure and the related accuracy of that measurement was based on a comparison of its observations with those from a nearby instrumented 300-m tower in Colorado (supplemented by instrumented airplane ascents above tower height), and also based on considerations of continuity in vertical profiles of Doppler system outputs. Input data requirements for dispersion models were then assessed. It is apparent that the Doppler system can provide all the approximate mean flow and turbulence factors used by the models, usually to altitudes beyond 600 m. There is also a need in the models for an input which is related to temperature stability, both for plume rise calculations, and for predicting vertical diffusion versus observed vertical turbulence. It is expected that a stability factor can be derived objectively from the Doppler acoustic signals; various candidate methods are discussed, but complete development of the technique is in the future.

  4. A discrete element and ray framework for rapid simulation of acoustical dispersion of microscale particulate agglomerations

    NASA Astrophysics Data System (ADS)

    Zohdi, T. I.

    2016-03-01

    In industry, particle-laden fluids, such as particle-functionalized inks, are constructed by adding fine-scale particles to a liquid solution, in order to achieve desired overall properties in both liquid and (cured) solid states. However, oftentimes undesirable particulate agglomerations arise due to some form of mutual-attraction stemming from near-field forces, stray electrostatic charges, process ionization and mechanical adhesion. For proper operation of industrial processes involving particle-laden fluids, it is important to carefully breakup and disperse these agglomerations. One approach is to target high-frequency acoustical pressure-pulses to breakup such agglomerations. The objective of this paper is to develop a computational model and corresponding solution algorithm to enable rapid simulation of the effect of acoustical pulses on an agglomeration composed of a collection of discrete particles. Because of the complex agglomeration microstructure, containing gaps and interfaces, this type of system is extremely difficult to mesh and simulate using continuum-based methods, such as the finite difference time domain or the finite element method. Accordingly, a computationally-amenable discrete element/discrete ray model is developed which captures the primary physical events in this process, such as the reflection and absorption of acoustical energy, and the induced forces on the particulate microstructure. The approach utilizes a staggered, iterative solution scheme to calculate the power transfer from the acoustical pulse to the particles and the subsequent changes (breakup) of the pulse due to the particles. Three-dimensional examples are provided to illustrate the approach.

  5. Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe1-xMxSi, M=Ir,Os

    DOE PAGES

    Delaire, O.; Al-Qasir, Iyad I.; May, Andrew F.; ...

    2015-03-31

    The vibrational behavior of heavy substitutional impurities (M=Ir,Os) in Fe1-xMxSi (x = 0, 0.02, 0.04, 0.1) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. In this paper, our INS measurements on single-crystals mapped the four-dimensional dynamical structure factor, S(Q;E), for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers and increases electron-phonon coupling, leads tomore » softened interatomic force-constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S(Q,E) from INS through a Green's function model incorporating the phonon self-energy based on first-principles density functional theory (DFT) simulations. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Finally, our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.« less

  6. Revealing the mechanism of passive transport in lipid bilayers via phonon-mediated nanometre-scale density fluctuations

    DOE PAGES

    Zhernenkov, Mikhail; Bolmatov, Dima; Soloviov, Dmitry; ...

    2016-05-12

    We report the high resolution inelastic x-ray study of the in-plane phonon excitations in dipalmitoyl phosphatidylcholine (DPPC) above and below main transition temperature. In the Lβ' gel phase, we observe high frequency longitudinal phonon mode previously predicted by the molecular dynamics simulations and for the first time, we reveal low frequency weakly dispersive transverse acoustic mode which softens and exhibits a low-frequency phonon gap when the DPPC lipid transitions into the Lα fluid phase. The phonon softening of the high frequency longitudinal excitations and the transformation of the transverse excitations upon the phase transition from the Lβ' to Lα phasemore » is explained within the framework of the phonon theory of liquids. These findings illustrate the importance of the collective dynamics of biomembranes and reveal that hydrocarbon tails can act as an efficient mediator in controlling the passive transport across the bilayer plane.« less

  7. Neutron inelastic scattering measurements of low-energy phonons in the multiferroic BiFeO3

    SciTech Connect

    Schneeloch, John A.; Xu, Zhijun; Wen, Jinsheng; Gehring, P. M.; Stock, C.; Matsuda, Masaaki; Winn, Barry L.; Gu, Genda; Shapiro, Stephen M.; Birgeneau, R. J.; Ushiyama, T.; Yanagisawa, Y.; Tomioka, Y.; Ito, T.; Xu, Guangyong

    2015-02-10

    In this study, we present neutron inelastic scattering measurements of the low-energy phonons in single crystal BiFeO3. The dispersions of the three acoustic phonon modes (LA along [100], TA1 along [010], and TA2 along [110]) and two low-energy optic phonon modes (LO and TO1) have been mapped out between 300 and 700 K. Elastic constants are extracted from the phonon measurements. The energy linewidths of both TA phonons at the zone boundary clearly broaden when the system is warmed toward the magnetic ordering temperature TN=640 K. In conclusion, this suggests that the magnetic order and low-energy lattice dynamics in this multiferroic material are coupled.

  8. Neutron inelastic scattering measurements of low-energy phonons in the multiferroic BiFeO3

    DOE PAGES

    Schneeloch, John A.; Xu, Zhijun; Wen, Jinsheng; ...

    2015-02-10

    In this study, we present neutron inelastic scattering measurements of the low-energy phonons in single crystal BiFeO3. The dispersions of the three acoustic phonon modes (LA along [100], TA1 along [010], and TA2 along [110]) and two low-energy optic phonon modes (LO and TO1) have been mapped out between 300 and 700 K. Elastic constants are extracted from the phonon measurements. The energy linewidths of both TA phonons at the zone boundary clearly broaden when the system is warmed toward the magnetic ordering temperature TN=640 K. In conclusion, this suggests that the magnetic order and low-energy lattice dynamics in thismore » multiferroic material are coupled.« less

  9. Negative refraction imaging of acoustic metamaterial lens in the supersonic range

    SciTech Connect

    Han, Jianning; Wen, Tingdun; Yang, Peng; Zhang, Lu

    2014-05-15

    Acoustic metamaterials with negative refraction index is the most promising method to overcome the diffraction limit of acoustic imaging to achieve ultrahigh resolution. In this paper, we use localized resonant phononic crystal as the unit cell to construct the acoustic negative refraction lens. Based on the vibration model of the phononic crystal, negative quality parameters of the lens are obtained while excited near the system resonance frequency. Simulation results show that negative refraction of the acoustic lens can be achieved when a sound wave transmiting through the phononic crystal plate. The patterns of the imaging field agree well with that of the incident wave, while the dispersion is very weak. The unit cell size in the simulation is 0.0005 m and the wavelength of the sound source is 0.02 m, from which we show that acoustic signal can be manipulated through structures with dimensions much smaller than the wavelength of incident wave.

  10. Phononic crystal diffraction gratings

    NASA Astrophysics Data System (ADS)

    Moiseyenko, Rayisa P.; Herbison, Sarah; Declercq, Nico F.; Laude, Vincent

    2012-02-01

    When a phononic crystal is interrogated by an external source of acoustic waves, there is necessarily a phenomenon of diffraction occurring on the external enclosing surfaces. Indeed, these external surfaces are periodic and the resulting acoustic diffraction grating has a periodicity that depends on the orientation of the phononic crystal. This work presents a combined experimental and theoretical study on the diffraction of bulk ultrasonic waves on the external surfaces of a 2D phononic crystal that consists of a triangular lattice of steel rods in a water matrix. The results of transmission experiments are compared with theoretical band structures obtained with the finite-element method. Angular spectrograms (showing frequency as a function of angle) determined from diffraction experiments are then compared with finite-element simulations of diffraction occurring on the surfaces of the crystal. The experimental results show that the diffraction that occurs on its external surfaces is highly frequency-dependent and has a definite relation with the Bloch modes of the phononic crystal. In particular, a strong influence of the presence of bandgaps and deaf bands on the diffraction efficiency is found. This observation opens perspectives for the design of efficient phononic crystal diffraction gratings.

  11. Splash, pop, sizzle: Information processing with phononic computing

    SciTech Connect

    Sklan, Sophia R.

    2015-05-15

    Phonons, the quanta of mechanical vibration, are important to the transport of heat and sound in solid materials. Recent advances in the fundamental control of phonons (phononics) have brought into prominence the potential role of phonons in information processing. In this review, the many directions of realizing phononic computing and information processing are examined. Given the relative similarity of vibrational transport at different length scales, the related fields of acoustic, phononic, and thermal information processing are all included, as are quantum and classical computer implementations. Connections are made between the fundamental questions in phonon transport and phononic control and the device level approach to diodes, transistors, memory, and logic. .

  12. Enhanced electron-phonon coupling for a semiconductor charge qubit in a surface phonon cavity

    PubMed Central

    Chen, J. C. H.; Sato, Y.; Kosaka, R.; Hashisaka, M.; Muraki, K.; Fujisawa, T.

    2015-01-01

    Electron-phonon coupling is a major decoherence mechanism, which often causes scattering and energy dissipation in semiconductor electronic systems. However, this electron-phonon coupling may be used in a positive way for reaching the strong or ultra-strong coupling regime in an acoustic version of the cavity quantum electrodynamic system. Here we propose and demonstrate a phonon cavity for surface acoustic waves, which is made of periodic metal fingers that constitute Bragg reflectors on a GaAs/AlGaAs heterostructure. Phonon band gap and cavity phonon modes are identified by frequency, time and spatially resolved measurements of the piezoelectric potential. Tunneling spectroscopy on a double quantum dot indicates the enhancement of phonon assisted transitions in a charge qubit. This encourages studying of acoustic cavity quantum electrodynamics with surface phonons. PMID:26469629

  13. Nonlinear control of high-frequency phonons in spider silk

    NASA Astrophysics Data System (ADS)

    Schneider, Dirk; Gomopoulos, Nikolaos; Koh, Cheong Y.; Papadopoulos, Periklis; Kremer, Friedrich; Thomas, Edwin L.; Fytas, George

    2016-10-01

    Spider dragline silk possesses superior mechanical properties compared with synthetic polymers with similar chemical structure due to its hierarchical structure comprised of partially crystalline oriented nanofibrils. To date, silk’s dynamic mechanical properties have been largely unexplored. Here we report an indirect hypersonic phononic bandgap and an anomalous dispersion of the acoustic-like branch from inelastic (Brillouin) light scattering experiments under varying applied elastic strains. We show the mechanical nonlinearity of the silk structure generates a unique region of negative group velocity, that together with the global (mechanical) anisotropy provides novel symmetry conditions for gap formation. The phononic bandgap and dispersion show strong nonlinear strain-dependent behaviour. Exploiting material nonlinearity along with tailored structural anisotropy could be a new design paradigm to access new types of dynamic behaviour.

  14. Low-concentration liquid sensing by an acoustic Mach-Zehnder interferometer in a two-dimensional phononic crystal

    NASA Astrophysics Data System (ADS)

    Salman, Aysevil; Adem Kaya, Olgun; Cicek, Ahmet; Ulug, Bulent

    2015-06-01

    Mach-Zehnder interferometer formed by liquid-filled linear defect waveguides in a two-dimensional phononic crystal is numerically realized for sensing low concentrations of an analyte. The waveguides in the square phononic crystal of void cylinders in steel, as well as their T branches and sharp bends are utilized to construct interferometer arms. Sensing low concentrations of ethanol on the order of 0.1% in a binary mixture with water is achieved by replacing the contents of a number of waveguide core cells on one arm of the interferometer with the analyte. Computations are carried out through the finite-element method in an approach that takes the solid-liquid interaction at the waveguide core cells into account. Band analyses reveal linear variation of the central frequency of the transmission band within a band gap for ethanol concentrations up to 3.0%. Phase difference due to the imbalance of the sample and reference arms of the interferometer also varies linearly with ethanol concentration, leading in turn to a cosine variation of the Fourier component of the temporal interferometer response at the central input-pulse frequency. The induced phase difference in the investigated configuration becomes a -0.78π and -0.65π per percent increase of ethanol concentration as calculated from the band-structure and transient data, respectively. This is confirmed by transient finite-element simulations where totally destructive interference occurs for a concentration of approximately 1.5%. The proposed scheme, which can easily be adopted to other binary mixtures, offers a compact implementation requiring small amounts of analyte.

  15. Measurement of Thermal Effects in the Dispersion Relation of the Dust Acoustic Wave

    NASA Astrophysics Data System (ADS)

    Hoyng, Joshua; Williams, Jeremiah

    2016-10-01

    A complex or dusty plasma is a four-component plasma system composed of ions, electrons, neutral particles and charged microparticles. The presence of these charged microparticles reveals different plasma phenomena, including a new wave mode known as the dust acoustic, or dust density, wave (DAW). The DAW is a low frequency, longitudinal mode that propagates through the microparticle component of the dusty plasma system and is self-excited by the energy from the ions streaming through this component. In recent years the DAW has been the subject of intense study and has provided a way to examine the thermal properties of the microparticle component. In this presentation, we report the results of an experimental study examining the thermal effects in the dispersion relation of this wave mode over a range of neutral gas pressures.

  16. Texture in steel plates revealed by laser ultrasonic surface acoustic waves velocity dispersion analysis.

    PubMed

    Yin, Anmin; Wang, Xiaochen; Glorieux, Christ; Yang, Quan; Dong, Feng; He, Fei; Wang, Yanlong; Sermeus, Jan; Van der Donck, Tom; Shu, Xuedao

    2017-02-24

    A photoacoustic, laser ultrasonics based approach in an Impulsive Stimulated Scattering (ISS) implementation was used to investigate the texture in polycrystalline metal plates. The angular dependence of the 'polycrystalline' surface acoustic wave (SAW) velocity measured along regions containing many grains was experimentally determined and compared with simulated results that were based on the angular dependence of the 'single grain' SAW velocity within single grains and the grain orientation distribution. The polycrystalline SAW velocities turn out to vary with texture. The SAW velocities and their angular variations for {110} texture were found to be larger than that the ones for {111} texture or the strong γ fiber texture. The SAW velocities for {001} texture were larger than for {111} texture, but with almost the same angular dependence. The results infer the feasibility to apply angular SAW angular dispersion measurements by laser ultrasonics for on-line texture monitoring.

  17. Fluid simulation of dispersive and nondispersive ion acoustic waves in the presence of superthermal electrons

    NASA Astrophysics Data System (ADS)

    Lotekar, Ajay; Kakad, Amar; Kakad, Bharati

    2016-10-01

    One-dimensional fluid simulation is performed for the unmagnetized plasma consisting of cold fluid ions and superthermal electrons. Such a plasma system supports the generation of ion acoustic (IA) waves. A standard Gaussian type perturbation is used in both electron and ion equilibrium densities to excite the IA waves. The evolutionary profiles of the IA waves are obtained by varying the superthermal index and the amplitude of the initial perturbation. This simulation demonstrates that the amplitude of the initial perturbation and the superthermal index play an important role in determining the time evolution and the characteristics of the generated IA waves. The initial density perturbation in the system creates charge separation that drives the finite electrostatic potential in the system. This electrostatic potential later evolves into the dispersive and nondispersive IA waves in the simulation system. The density perturbation with the amplitude smaller than 10% of the equilibrium plasma density evolves into the dispersive IA waves, whereas larger density perturbations evolve into both dispersive and nondispersive IA waves for lower and higher superthermal index. The dispersive IA waves are the IA oscillations that propagate with constant ion plasma frequency, whereas the nondispersive IA waves are the IA solitary pulses (termed as IA solitons in the stability region) that propagate with the constant wave speed. The characteristics of the stable nondispersive IA solitons are found to be consistent with the nonlinear fluid theory. To the best of our knowledge, this is the first fluid simulation study that has considered the superthermal distributions for the plasma species to model the electrostatic solitary waves.

  18. Femtosecond electron imaging of defect-modulated phonon dynamics

    PubMed Central

    Cremons, Daniel R.; Plemmons, Dayne A.; Flannigan, David J.

    2016-01-01

    Precise manipulation and control of coherent lattice oscillations via nanostructuring and phonon-wave interference has the potential to significantly impact a broad array of technologies and research areas. Resolving the dynamics of individual phonons in defect-laden materials presents an enormous challenge, however, owing to the interdependent nanoscale and ultrafast spatiotemporal scales. Here we report direct, real-space imaging of the emergence and evolution of acoustic phonons at individual defects in crystalline WSe2 and Ge. Via bright-field imaging with an ultrafast electron microscope, we are able to image the sub-picosecond nucleation and the launch of wavefronts at step edges and resolve dispersion behaviours during propagation and scattering. We discover that the appearance of speed-of-sound (for example, 6 nm ps−1) wavefronts are influenced by spatially varying nanoscale strain fields, taking on the appearance of static bend contours during propagation. These observations provide unprecedented insight into the roles played by individual atomic and nanoscale features on acoustic-phonon dynamics. PMID:27079790

  19. Methods for the treatment of acoustic and absorptive/dispersive wave field measurements

    NASA Astrophysics Data System (ADS)

    Innanen, Kristopher Albert Holm

    Many recent methods of seismic wave field processing and inversion concern themselves with the fine detail of the amplitude and phase characteristics of measured events. Processes of absorption and dispersion have a strong impact on both; the impact is particularly deleterious to the effective resolution of images created from the data. There is a need to understand the dissipation of seismic wave energy as it affects such methods. I identify: algorithms based on the inverse scattering series, algorithms based on multiresolution analysis, and algorithms based on the estimation of the order of the singularities of seismic data, as requiring this kind of study. As it turns out, these approaches may be cast such that they deal directly with issues of attenuation, to the point where they can be seen as tools for viscoacoustic forward modelling, Q estimation; viscoacoustic inversion, and/or Q compensation. In this thesis I demonstrate these ideas in turn. The forward scattering series is formulated such that a viscoacoustic wave field is represented as an expansion about an acoustic reference; analysis of the convergence properties and scattering diagrams are carried out, and it is shown that (i) the attenuated wave field may be generated by the nonlinear interplay of acoustic reference fields, and (ii) the cumulative effect of certain scattering types is responsible for macroscopic wave field properties: also, the basic form of the absorptive/dispersive inversion problem is predicted. Following this, the impact of Q on measurements of the local regularity of a seismic trace, via Lipschitz exponents, is discussed, with the aim of using these exponents as a means to estimate local Q values. The problem of inverse scattering based imaging and inversion is treated next: I present a simple, computable form for the simultaneous imaging and wavespeed inversion of 1D acoustic wave field data. This method is applied to 1D, normal incidence synthetic data: its sensitivity with

  20. Preserving the Helmholtz dispersion relation: One-way acoustic wave propagation using matrix square roots

    NASA Astrophysics Data System (ADS)

    Keefe, Laurence

    2016-11-01

    Parabolized acoustic propagation in transversely inhomogeneous media is described by the operator update equation U (x , y , z + Δz) =eik0 (- 1 +√{ 1 + Z }) U (x , y , z) for evolution of the envelope of a wavetrain solution to the original Helmholtz equation. Here the operator, Z =∇T2 + (n2 - 1) , involves the transverse Laplacian and the refractive index distribution. Standard expansion techniques (on the assumption Z << 1)) produce pdes that approximate, to greater or lesser extent, the full dispersion relation of the original Helmholtz equation, except that none of them describe evanescent/damped waves without special modifications to the expansion coefficients. Alternatively, a discretization of both the envelope and the operator converts the operator update equation into a matrix multiply, and existing theorems on matrix functions demonstrate that the complete (discrete) Helmholtz dispersion relation, including evanescent/damped waves, is preserved by this discretization. Propagation-constant/damping-rates contour comparisons for the operator equation and various approximations demonstrate this point, and how poorly the lowest-order, textbook, parabolized equation describes propagation in lined ducts.

  1. Modulations of thermal properties of graphene by strain-induced phonon engineering

    NASA Astrophysics Data System (ADS)

    Tada, Kento; Funatani, Takashi; Konabe, Satoru; Sasaoka, Kenji; Ogawa, Matsuto; Souma, Satofumi; Yamamoto, Takahiro

    2017-02-01

    Modulation of the thermal properties of graphene due to strain-induced phononic band engineering was theoretically investigated by first-principles calculations based on the density functional theory. The high-energy phonon modes are found to exhibit softening owing to the strain, whereas a low-energy acoustic mode (out-of-plane mode) exhibits hardening. Moreover, the dispersion relation of the out-of-plane mode associated with the strain essentially changes from quadratic (∝ k 2) to linear (∝ k). Accordingly, the temperature dependence of the low-temperature specific heat also changes from linear (∝ T) to quadratic (∝ T 2).

  2. Using coupling slabs to tailor surface-acoustic-wave band structures in phononic crystals consisting of pillars attached to elastic substrates

    NASA Astrophysics Data System (ADS)

    Zhang, Heng; Yu, SiYuan; Liu, FuKang; Wang, Zhen; Lu, MingHui; Hu, XiaoBo; Chen, YanFeng; Xu, XianGang

    2017-04-01

    The propagation of surface acoustic waves (SAWs) in two-dimensional phononic crystals (PnCs) with and without coupling-enhancement slabs was theoretically investigated using a three-dimensional finite element method. Different piezoelectric substrates, for example, lithium niobate (LiNbO3), gallium nitride (GaN), and aluminium nitride (AlN), were taken into account. Compared to the PnCs without coupling-enhancement slabs, the coupling between each pillar and its nearest neighbor was largely enhanced in the presence of slabs. The bandwidth of the first directional band gap increased markedly compared with its initial value for the PnCs without a slab (within square symmetry). In addition, with increasing thicknesses of the slabs bonded between neighboring pillars, the first directional band-gap and second directional band gap of the PnCs tend to merge. Therefore, the structure with coupling-enhancement slabs can be used as an excellent electrical band elimination filter for most electro-SAW devices, offering a new strategy to realize chip-scale applications in electroacoustic signal processing, optoacoustic modulation, and even SAW microfluidic devices.

  3. Hawking Radiation from an Acoustic Black Hole on an Ion Ring

    SciTech Connect

    Horstmann, B.; Cirac, J. I.; Reznik, B.; Fagnocchi, S.

    2010-06-25

    In this Letter we propose to simulate acoustic black holes with ions in rings. If the ions are rotating with a stationary and inhomogeneous velocity profile, regions can appear where the ion velocity exceeds the group velocity of the phonons. In these regions phonons are trapped like light in black holes, even though we have a discrete field theory and a nonlinear dispersion relation. We study the appearance of Hawking radiation in this setup and propose a scheme to detect it.

  4. Sound and heat revolutions in phononics.

    PubMed

    Maldovan, Martin

    2013-11-14

    The phonon is the physical particle representing mechanical vibration and is responsible for the transmission of everyday sound and heat. Understanding and controlling the phononic properties of materials provides opportunities to thermally insulate buildings, reduce environmental noise, transform waste heat into electricity and develop earthquake protection. Here I review recent progress and the development of new ideas and devices that make use of phononic properties to control both sound and heat. Advances in sonic and thermal diodes, optomechanical crystals, acoustic and thermal cloaking, hypersonic phononic crystals, thermoelectrics, and thermocrystals herald the next technological revolution in phononics.

  5. Preface: Phonons 2007

    NASA Astrophysics Data System (ADS)

    Perrin, Bernard

    2007-06-01

    Conference logo The conference PHONONS 2007 was held 15-20 July 2007 in the Conservatoire National des Arts et Métiers (CNAM) Paris, France. CNAM is a college of higher technology for training students in the application of science to industry, founded by Henri Grégoire in 1794. This was the 12th International Conference on Phonon Scattering in Condensed Matter. This international conference series, held every 3 years, started in France at Sainte-Maxime in 1972. It was then followed by meetings at Nottingham (1975), Providence (1979), Stuttgart (1983), Urbana-Champaign (1986), Heidelberg (1989), Ithaca (1992), Sapporo (1995), Lancaster (1998), Dartmouth (2001) and St Petersburg (2004). PHONONS 2007 was attended by 346 delegates from 37 different countries as follows: France 120, Japan 45, Germany 25, USA 25, Russia 21, Italy 13, Poland 9, UK 9, Canada 7, The Netherlands 7, Finland 6, Spain 6, Taiwan 6, Greece 4, India 4, Israel 4, Ukraine 4, Serbia 3, South Africa 3, Argentina 2, Belgium 2, China 2, Iran 2, Korea 2, Romania 2, Switzerland 2, and one each from Belarus, Bosnia-Herzegovina, Brazil, Bulgaria, Egypt, Estonia, Mexico, Moldova, Morocco, Saudi Arabia, Turkey. There were 5 plenary lectures, 14 invited talks and 84 oral contributions; 225 posters were presented during three poster sessions. The first plenary lecture was given by H J Maris who presented fascinating movies featuring the motion of a single electron in liquid helium. Robert Blick gave us a review on the new possibilities afforded by nanotechnology to design nano-electomechanical systems (NEMS) and the way to use them to study elementary and fundamental processes. The growing interest for phonon transport studies in nanostructured materials was demonstrated by Arun Majumdar. Andrey Akimov described how ultrafast acoustic solitons can monitor the optical properties of quantum wells. Finally, Maurice Chapellier told us how

  6. Phonon thermal properties of graphene from molecular dynamics using different potentials

    NASA Astrophysics Data System (ADS)

    Zou, Ji-Hang; Ye, Zhen-Qiang; Cao, Bing-Yang

    2016-10-01

    Phonon thermal transport in graphene has attracted significant interest in recent years. Phonon thermal properties of graphene are investigated by molecular dynamics simulations using the Tersoff, Tersoff-2010, REBO, and AIREBO potentials. By calculating the phonon properties and thermal conductivity of graphene, the performance of the potentials is evaluated based on comparisons with experimental data. It shows that the Tersoff-2010 and REBO display better dispersion curves for graphene than the original Tersoff and AIREBO. The Tersoff-2010 correctly provides the Γ point phonon velocities of the LA and TA branches as well as the G peak frequency with a value of 46 THz. In addition, the acoustic phonon relaxation time derived from the Tersoff-2010 satisfies the ideal relation "τ-1 ∝ ν2." It is also found that the Tersoff-2010 provides the highest graphene thermal conductivity among the used potentials, and estimates about 30.0% contribution for flexural phonons to the total thermal conductivity. By comparison, the Tersoff-2010 potential is demonstrated to be the most suitable one to describe the phonon thermal properties of graphene.

  7. Dispersion relations for surface excitations as a probe for variational solutions of optimized paired-phonon analysis equations

    NASA Astrophysics Data System (ADS)

    Szybisz, Leszek

    1990-06-01

    The self-consistency of solutions obtained from a recently proposed numerical relaxation method of solving the Euler-Lagrange equations for the ground state of inhomogeneous Bose systems at zero temperature is investigated. For this kind of system at least three different dispersion relations can be formulated, all of them providing information about the same eigenstates. The quality of our optimization scheme is studied by analyzing the convergence of the low-lying eigenvalues and eigenfunctions of these dispersion relations. Numerical results for the spectrum and spatial shape of elementary excitations of a thin film of liquid 4He supported by an external potential are reported. The optimal lowest-lying eigenvalues are compared with estimations based on simple theoretical approaches and with calculations performed by other authors.

  8. Gaseous Absorption and Dispersion of Sound in a Resonant Cylindrical Cavity: AN Acoustic and Photoacoustic Study

    NASA Astrophysics Data System (ADS)

    Beckwith, Clyfe Gordon

    This research investigated the feasibility of accurately measuring Virial coefficients in an acoustically resonant cylindrical cavity. Gases studied were: Argon, Helium, Nitrogen, Carbon Dioxide, and Methane. Parameters considered were: resonant frequencies (f_ {rm r}- also a measure of speed of sound), quality factors (Q), and signal amplitudes. We studied the longitudinal modes smaller than 2000 Hz, at room temperature and at pressures of 200, 500, and 800 mm of Hg. The choice of the longitudinal modes was predetermined by our wish to compare acoustic and photoacoustic resonance techniques of the same mode. The acoustic excitation is limited to the longitudinal modes and is achieved by placing a loudspeaker close to one end of the cavity. Photoacoustically we excite a small concentration of molecular Iodine, mixed in with the buffer gases, by a periodically interrupted Xenon light beam. By increasing the length of the cavity we could decrease the space between the modes of frequency. Our observations focused on the behaviors that (a) f_{rm r} shifted with pressure, (b) the f_{rm r} deviated from the simple laws of harmonics, and (c) the amplitudes for the two techniques varied differently with frequency. Effect (a) is due to the fact that the gases are not "ideal", and due to the presence of boundary layers caused by thermal conduction and viscosity gradients. Effect (b) arises because of the f_{rm r}'s mode dependence, caused by the wave scattering due to imperfect geometrical symmetries. Effect (c) is governed by the coupling factors. All measurements could theoretically be justified to within instrumental error, the only noted discrepancy is the lack of a theoretical mode dependence. We conclude that it is feasible to study the accuracy of Virial coefficients of simple gases provided that the boundary layer loss effects and the mode dependent wave scattering can be quantified; in regions of high pressures and high frequencies the Virial effects dominate the

  9. Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe1-xMxSi, M=Ir,Os

    SciTech Connect

    Delaire, O.; Al-Qasir, Iyad I.; May, Andrew F.; Sales, Brian C.; Niedziela, Jennifer L.; Ma, Jie; Matsuda, Masaaki; Abernathy, Douglas L.; Berlijn, Tom

    2015-03-31

    The vibrational behavior of heavy substitutional impurities (M=Ir,Os) in Fe1-xMxSi (x = 0, 0.02, 0.04, 0.1) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. In this paper, our INS measurements on single-crystals mapped the four-dimensional dynamical structure factor, S(Q;E), for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers and increases electron-phonon coupling, leads to softened interatomic force-constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S(Q,E) from INS through a Green's function model incorporating the phonon self-energy based on first-principles density functional theory (DFT) simulations. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Finally, our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.

  10. Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe1-xMxSi (M =Ir , Os )

    NASA Astrophysics Data System (ADS)

    Delaire, O.; Al-Qasir, I. I.; May, A. F.; Li, C. W.; Sales, B. C.; Niedziela, J. L.; Ma, J.; Matsuda, M.; Abernathy, D. L.; Berlijn, T.

    2015-03-01

    The vibrational behavior of heavy substitutional impurities (M = Ir,Os) in Fe1-xMxSi (x =0 ,0.02 ,0.04 ,0.1 ) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. Our INS measurements on single crystals mapped the four-dimensional dynamical structure factor, S (Q ,E ) , for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers, leads to softened interatomic force constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S (Q ,E ) from INS through a Green's-function model incorporating the phonon self-energy based on first-principles density functional theory simulations, and we study the disorder-induced lifetimes on large supercells. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.

  11. Bendable Electro-Acoustic Transducer Fabricated Utilizing Frequency Dispersion of Elastic Modulus

    NASA Astrophysics Data System (ADS)

    Miyoshi, Tetsu; Ohga, Juro

    2013-09-01

    To realize the speaker diaphragm that can be united with a flexible display without deteriorating lightweight properties and flexibility, a novel bendable electro-acoustic transducer (BEAT) based on 0-3-type piezoelectric composites has been developed. To overcome the trade-off between flexibility and the transmission efficiency of vibration energy, a viscoelastic polymer that has local maximum points in the loss factor as well as large frequency dispersion in the storage modulus near room temperature was employed as the matrix of the piezoelectric composite layer. Against the comparatively slow (10 Hz or less) deformation from the outside, the viscoelastic matrix is viscous enough to prevent cracking and delamination. On the other hand, in the audible range (20 Hz to 20 kHz), the matrix is elastic enough to transmit piezoelectric vibration energy, maintaining a moderately large loss factor as well as a high sound velocity. For the first time, we successfully demonstrated a rollable speaker that can continue to generate a high-quality sound while being rolled and unrolled repeatedly onto a cylinder with a curvature radius of 4 mm.

  12. Low-Dispersion Scheme for Nonlinear Acoustic Waves in Nonuniform Flow

    NASA Technical Reports Server (NTRS)

    Baysal, Oktay; Kaushik, Dinesh K.; Idres, Moumen

    1997-01-01

    The linear dispersion-relation-preserving scheme and its boundary conditions have been extended to the nonlinear Euler equations. This allowed computing, a nonuniform flowfield and a nonlinear acoustic wave propagation in such a medium, by the same scheme. By casting all the equations, boundary conditions, and the solution scheme in generalized curvilinear coordinates, the solutions were made possible for non-Cartesian domains and, for the better deployment of the grid points, nonuniform grid step sizes could be used. It has been tested for a number of simple initial-value and periodic-source problems. A simple demonstration of the difference between a linear and nonlinear propagation was conducted. The wall boundary condition, derived from the momentum equations and implemented through a pressure at a ghost point, and the radiation boundary condition, derived from the asymptotic solution to the Euler equations, have proven to be effective for the nonlinear equations and nonuniform flows. The nonreflective characteristic boundary conditions also have shown success but limited to the nonlinear waves in no mean flow, and failed for nonlinear waves in nonuniform flow.

  13. Al2C Monolayer Sheet and Nanoribbons with Unique Direction-Dependent Acoustic-Phonon-Limited Carrier Mobility and Carrier Polarity.

    PubMed

    Xu, Yuehua; Dai, Jun; Zeng, Xiao Cheng

    2016-01-21

    The intrinsic acoustic-phonon-limited carrier mobility (μ) of Al2C monolayer sheet and nanoribbons are investigated using ab initio computation and deformation potential theory. It is found that the polarity of the room-temperature carrier mobility of the Al2C monolayer is direction-dependent, with μ of electron (e) and hole (h) being 2348 and 40.77 cm(2)/V/s, respectively, in the armchair direction and 59.95 (e) and 705.8 (h) in the zigzag direction. More interestingly, one-dimensional Al2C nanoribbons not only can retain the direction-dependent polarity but also may entail even higher mobility, in contrast to either the graphene nanoribbons which tend to exhibit lower μ compared to the two-dimensional graphene or the MoS2 nanoribbons which have reversed polarity compared to the MoS2 sheet. As an example, the Al-terminated zigzag nanoribbon with a width of 4.1 nm exhibits μ of 212.6 (e) and 2087 (h) cm(2)/V/s, while the C-terminated armchair nanoribbon with a width 2.6 nm exhibits μ of 1090 (e) and 673.9 (h) cm(2)/V/s; the C-terminated zigzag nanoribbon with a width 3.7 nm exhibits μ of 177.6 (e) and 1889 (h) cm(2)/V/s, and the Al-terminated armchair nanoribbon with a width 2.4 nm exhibits μ of 6695 (e) and 518.4 (h) cm(2)/V/s. The high carrier mobility, μ, coupled with polarity and direction dependence endows the Al2C sheet and nanoribbons with unique transport properties that can be exploited for special applications in nanoelectronics.

  14. Microfabricated phononic crystal devices and applications

    NASA Astrophysics Data System (ADS)

    Olsson, R. H., III; El-Kady, I.

    2009-01-01

    Phononic crystals are the acoustic wave analogue of photonic crystals. Here a periodic array of scattering inclusions located in a homogeneous host material forbids certain ranges of acoustic frequencies from existence within the crystal, thus creating what are known as acoustic bandgaps. The majority of previously reported phononic crystal devices have been constructed by hand, assembling scattering inclusions in a viscoelastic medium, predominantly air, water or epoxy, resulting in large structures limited to frequencies below 1 MHz. Recently, phononic crystals and devices have been scaled to VHF (30-300 MHz) frequencies and beyond by utilizing microfabrication and micromachining technologies. This paper reviews recent developments in the area of micro-phononic crystals including design techniques, material considerations, microfabrication processes, characterization methods and reported device structures. Micro-phononic crystal devices realized in low-loss solid materials are emphasized along with their potential application in radio frequency communications and acoustic imaging for medical ultrasound and nondestructive testing. The reported advances in batch micro-phononic crystal fabrication and simplified testing promise not only the deployment of phononic crystals in a number of commercial applications but also greater experimentation on a wide variety of phononic crystal structures.

  15. Slow light and broadband coherent phonon generation

    NASA Astrophysics Data System (ADS)

    Wang, Zheng; Rakich, Peter; Reinke, Charles; Camacho, Ryan; Davids, Paul

    2012-03-01

    Recent advance in controlling optical forces using nanostructures suggests that nanoscale optical waveguides are capable of generating coherent acoustic phonons efficiently through a combination of radiation pressure and electrostriction. We discuss the critical roles of group velocity in such processes. This photon-phonon coupling would allow an acoustic intermediary to perform on-chip optical delay with a capacity 105 greater than photonic delay lines of the same size.

  16. Coherent phonon optics in a chip with an electrically controlled active device.

    PubMed

    Poyser, Caroline L; Akimov, Andrey V; Campion, Richard P; Kent, Anthony J

    2015-02-05

    Phonon optics concerns operations with high-frequency acoustic waves in solid media in a similar way to how traditional optics operates with the light beams (i.e. photons). Phonon optics experiments with coherent terahertz and sub-terahertz phonons promise a revolution in various technical applications related to high-frequency acoustics, imaging, and heat transport. Previously, phonon optics used passive methods for manipulations with propagating phonon beams that did not enable their external control. Here we fabricate a phononic chip, which includes a generator of coherent monochromatic phonons with frequency 378 GHz, a sensitive coherent phonon detector, and an active layer: a doped semiconductor superlattice, with electrical contacts, inserted into the phonon propagation path. In the experiments, we demonstrate the modulation of the coherent phonon flux by an external electrical bias applied to the active layer. Phonon optics using external control broadens the spectrum of prospective applications of phononics on the nanometer scale.

  17. Coherent phonon optics in a chip with an electrically controlled active device

    PubMed Central

    Poyser, Caroline L.; Akimov, Andrey V.; Campion, Richard P.; Kent, Anthony J.

    2015-01-01

    Phonon optics concerns operations with high-frequency acoustic waves in solid media in a similar way to how traditional optics operates with the light beams (i.e. photons). Phonon optics experiments with coherent terahertz and sub-terahertz phonons promise a revolution in various technical applications related to high-frequency acoustics, imaging, and heat transport. Previously, phonon optics used passive methods for manipulations with propagating phonon beams that did not enable their external control. Here we fabricate a phononic chip, which includes a generator of coherent monochromatic phonons with frequency 378 GHz, a sensitive coherent phonon detector, and an active layer: a doped semiconductor superlattice, with electrical contacts, inserted into the phonon propagation path. In the experiments, we demonstrate the modulation of the coherent phonon flux by an external electrical bias applied to the active layer. Phonon optics using external control broadens the spectrum of prospective applications of phononics on the nanometer scale. PMID:25652241

  18. Strong coupling between phonons and optical beating in backward Brillouin scattering

    NASA Astrophysics Data System (ADS)

    Huy, Kien Phan; Beugnot, Jean-Charles; Tchahame, Joël-Cabrel; Sylvestre, Thibaut

    2016-10-01

    Brillouin scattering is a fundamental nonlinear interaction between two optical waves and an acoustic wave mediated by electrostriction and photoelasticity. In this paper, we revisit the usual theory of this inelastic scattering to get a joint system in which the acoustic wave is strongly coupled to the interference pattern between the optical waves. We show in particular that when the coupling rate exceeds the phonon damping rate, the system enters the strong-coupling regime, giving rise to anticrossing in the dispersion relation and Rabi-like splitting. We further find numerically that strong coupling can, in principle, be observed using backward Brillouin scattering in subwavelength-diameter optical waveguides.

  19. Electron-phonon superconductivity in BaSn5

    NASA Astrophysics Data System (ADS)

    Billington, David; Ernsting, David; Millichamp, Thomas E.; Dugdale, Stephen B.

    2015-05-01

    First-principles calculations of the electronic structure and phonon dispersion relation of the superconducting compound ? were performed. This has allowed the calculation of the electron-phonon matrix elements from which the electron-phonon coupling constant was found to be ?. Application of the Allen-Dynes formula with ? yielded a superconducting transition temperature of ? K. The calculated ? agrees well with the available experimental data and indicates that ? is an electron-phonon superconductor with intermediate strength electron-phonon coupling.

  20. Off-axis phonon and photon propagation in porous silicon superlattices studied by Brillouin spectroscopy and optical reflectance

    SciTech Connect

    Parsons, L. C. Andrews, G. T.

    2014-07-21

    Brillouin light scattering experiments and optical reflectance measurements were performed on a pair of porous silicon-based optical Bragg mirrors which had constituent layer porosity ratios close to unity. For off-axis propagation, the phononic and photonic band structures of the samples were modeled as a series of intersecting linear dispersion curves. Zone-folding was observed for the longitudinal bulk acoustic phonon and the frequency of the probed zone-folded longitudinal phonon was shown to be dependent on the propagation direction as well as the folding order of the mode branch. There was no conclusive evidence of coupling between the transverse and the folded longitudinal modes. Two additional observed Brillouin peaks were attributed to the Rayleigh surface mode and a possible pseudo-surface mode. Both of these modes were dispersive, with the velocity increasing as the wavevector decreased.

  1. Second Harmonic Generation of Nanoscale Phonon Wave Packets.

    PubMed

    Bojahr, A; Gohlke, M; Leitenberger, W; Pudell, J; Reinhardt, M; von Reppert, A; Roessle, M; Sander, M; Gaal, P; Bargheer, M

    2015-11-06

    Phonons are often regarded as delocalized quasiparticles with certain energy and momentum. The anharmonic interaction of phonons determines macroscopic properties of the solid, such as thermal expansion or thermal conductivity, and a detailed understanding becomes increasingly important for functional nanostructures. Although phonon-phonon scattering processes depicted in simple wave-vector diagrams are the basis of theories describing these macroscopic phenomena, experiments directly accessing these coupling channels are scarce. We synthesize monochromatic acoustic phonon wave packets with only a few cycles to introduce nonlinear phononics as the acoustic counterpart to nonlinear optics. Control of the wave vector, bandwidth, and consequently spatial extent of the phonon wave packets allows us to observe nonlinear phonon interaction, in particular, second harmonic generation, in real time by wave-vector-sensitive Brillouin scattering with x-rays and optical photons.

  2. Low temperature phonon-drag thermopower in a monolayer MoS{sub 2}

    SciTech Connect

    Bhargavi, K. S. Kubakaddi, S. S.

    2015-06-24

    Phonon-drag thermopower S{sup g} is studied theoretically in a monolayer MoS{sub 2} as a function of temperature T. Electron-acoustic phonon (el-ap) interaction via deformation potential (DP) coupling of TA (LA) phonons is taken to be unscreened (screened) and piezoelectric (PE) coupling of LA and TA phonons is taken to be screened. S{sup g} due to DP coupling of TA phonons is found to be dominant over all other mechanisms. In the Bloch-Gruneisen (BG) regime power law S{sup g} ∼ T{sup 3} (T {sup 5}) is predicted for unscreened (screened) el-ap interaction a characteristic of two-dimensional phonons with linear dispersion. Screening strongly suppresses S{sup g} due to large effective mass of the electrons. We find that, S{sup g} due to screened DP and PE couplings are nearly same in contrast with the results in GaAs heterojunctions. With the increasing T its exponent decreases and reaches a sublinear value.

  3. Analytic studies of dispersive properties of shear Alfvén and acoustic wave spectra in tokamaks

    SciTech Connect

    Chavdarovski, Ilija; Zonca, Fulvio

    2014-05-15

    The properties of the low frequency shear Alfvén and acoustic wave spectra in toroidal geometry are examined analytically and numerically considering wave particle interactions with magnetically trapped and circulating particles, using the theoretical model described in [I. Chavdarovski and F. Zonca, Plasma Phys. Controlled Fusion 51, 115001 (2009)] and following the framework of the generalized fishbone-like dispersion relation. Effects of trapped particles as well as diamagnetic effects on the frequencies and damping rates of the beta-induced Alfvén eigenmodes, kinetic ballooning modes and beta-induced Alfvén-acoustic eigenmodes are discussed and shown to be crucial to give a proper assessment of mode structure and stability conditions. Present results also demonstrate the mutual coupling of these various branches and suggest that frequency as well as mode polarization are crucial for their identification on the basis of experimental evidence.

  4. Analytic studies of dispersive properties of shear Alfvén and acoustic wave spectra in tokamaks

    NASA Astrophysics Data System (ADS)

    Chavdarovski, Ilija; Zonca, Fulvio

    2014-05-01

    The properties of the low frequency shear Alfvén and acoustic wave spectra in toroidal geometry are examined analytically and numerically considering wave particle interactions with magnetically trapped and circulating particles, using the theoretical model described in [I. Chavdarovski and F. Zonca, Plasma Phys. Controlled Fusion 51, 115001 (2009)] and following the framework of the generalized fishbone-like dispersion relation. Effects of trapped particles as well as diamagnetic effects on the frequencies and damping rates of the beta-induced Alfvén eigenmodes, kinetic ballooning modes and beta-induced Alfvén-acoustic eigenmodes are discussed and shown to be crucial to give a proper assessment of mode structure and stability conditions. Present results also demonstrate the mutual coupling of these various branches and suggest that frequency as well as mode polarization are crucial for their identification on the basis of experimental evidence.

  5. Temperature Dependence of Phonons in Pyrolitic Graphite

    DOE R&D Accomplishments Database

    Brockhouse, B. N.; Shirane, G.

    1977-01-01

    Dispersion curves for longitudinal and transverse phonons propagating along and near the c-axis in pyrolitic graphite at temperatures between 4°K and 1500°C have been measured by neutron spectroscopy. The observed frequencies decrease markedly with increasing temperature (except for the transverse optical ''rippling'' modes in the hexagonal planes). The neutron groups show interesting asymmetrical broadening ascribed to interference between one phonon and many phonon processes.

  6. Spatial and temporal frequency domain laser-ultrasound applied in the direct measurement of dispersion relations of surface acoustic waves

    NASA Astrophysics Data System (ADS)

    Grünsteidl, Clemens; Veres, István A.; Roither, Jürgen; Burgholzer, Peter; Murray, Todd W.; Berer, Thomas

    2013-01-01

    We present a laser-ultrasound measurement technique which combines adjustable spatial and temporal modulation of the excitation laser beam. Our method spreads the intensity of an amplitude modulated continuous wave laser over a micro-scale pattern on the sample surface to excite surface acoustic waves. The excitation pattern consists of parallel, equidistant lines and the waves generated from the individual lines interfere on the sample surface. Measurement is done in the spatial-temporal frequency domain allowing the direct determination of dispersion relations. The technique performs with high signal-to-noise-ratios and low peak power densities on the sample.

  7. A New Wave of Acoustics.

    ERIC Educational Resources Information Center

    Beyer, Robert

    1981-01-01

    Surveys 50 years of acoustical studies by discussing selected topics including the ear, nonlinear representations, underwater sound, acoustical diagnostics, absorption, electrolytes, phonons, magnetic interaction, and superfluidity and the five sounds. (JN)

  8. Nonlinear ultrafast acoustics at the nano scale.

    PubMed

    van Capel, P J S; Péronne, E; Dijkhuis, J I

    2015-02-01

    Pulsed femtosecond lasers can generate acoustic pulses propagating in solids while displaying either diffraction, attenuation, nonlinearity and/or dispersion. When acoustic attenuation and diffraction are negligible, shock waves or solitons can form during propagation. Both wave types are phonon wavepackets with characteristic length scales as short as a few nanometer. Hence, they are well suited for acoustic characterization and manipulation of materials on both ultrafast and ultrashort scales. This work presents an overview of nonlinear ultrasonics since its first experimental demonstration at the beginning of this century to the more recent developments. We start by reviewing the main properties of nonlinear ultrafast acoustic propagation based on the underlying equations. Then we show various results obtained by different groups around the world with an emphasis on recent work. Current issues and directions of future research are discussed.

  9. Phonon spectroscopy with sub-meV resolution by femtosecond x-ray diffuse scattering

    DOE PAGES

    Zhu, Diling; Robert, Aymeric; Henighan, Tom; ...

    2015-08-10

    We present a reconstruction of the transverse acoustic phonon dispersion of germanium from femtosecond time-resolved x-ray diffuse scattering measurements at the Linac Coherent Light Source. We demonstrate an energy resolution of 0.3 meV with a momentum resolution of 0.01 nm-1 using 10-keV x rays with a bandwidth of ~ 1 eV. This high resolution was achieved simultaneously for a large section of reciprocal space including regions closely following three of the principal symmetry directions. The phonon dispersion was reconstructed with less than 3 h of measurement time, during which neither the x-ray energy, the sample orientation, nor the detector positionmore » were scanned. In conclusion, these results demonstrate how time-domain measurements can complement conventional frequency domain inelastic-scattering techniques.« less

  10. Phonon spectroscopy with sub-meV resolution by femtosecond x-ray diffuse scattering

    SciTech Connect

    Zhu, Diling; Robert, Aymeric; Lemke, Henrik T.; Trigo, Mariano

    2015-08-10

    We present a reconstruction of the transverse acoustic phonon dispersion of germanium from femtosecond time-resolved x-ray diffuse scattering measurements at the Linac Coherent Light Source. We demonstrate an energy resolution of 0.3 meV with a momentum resolution of 0.01 nm-1 using 10-keV x rays with a bandwidth of ~ 1 eV. This high resolution was achieved simultaneously for a large section of reciprocal space including regions closely following three of the principal symmetry directions. The phonon dispersion was reconstructed with less than 3 h of measurement time, during which neither the x-ray energy, the sample orientation, nor the detector position were scanned. In conclusion, these results demonstrate how time-domain measurements can complement conventional frequency domain inelastic-scattering techniques.

  11. Acoustics

    NASA Technical Reports Server (NTRS)

    Goodman, Jerry R.; Grosveld, Ferdinand

    2007-01-01

    The acoustics environment in space operations is important to maintain at manageable levels so that the crewperson can remain safe, functional, effective, and reasonably comfortable. High acoustic levels can produce temporary or permanent hearing loss, or cause other physiological symptoms such as auditory pain, headaches, discomfort, strain in the vocal cords, or fatigue. Noise is defined as undesirable sound. Excessive noise may result in psychological effects such as irritability, inability to concentrate, decrease in productivity, annoyance, errors in judgment, and distraction. A noisy environment can also result in the inability to sleep, or sleep well. Elevated noise levels can affect the ability to communicate, understand what is being said, hear what is going on in the environment, degrade crew performance and operations, and create habitability concerns. Superfluous noise emissions can also create the inability to hear alarms or other important auditory cues such as an equipment malfunctioning. Recent space flight experience, evaluations of the requirements in crew habitable areas, and lessons learned (Goodman 2003; Allen and Goodman 2003; Pilkinton 2003; Grosveld et al. 2003) show the importance of maintaining an acceptable acoustics environment. This is best accomplished by having a high-quality set of limits/requirements early in the program, the "designing in" of acoustics in the development of hardware and systems, and by monitoring, testing and verifying the levels to ensure that they are acceptable.

  12. Three material and four material one-dimensional phononic crystals

    NASA Astrophysics Data System (ADS)

    Kriegel, Ilka; Scotognella, Francesco

    2017-01-01

    In this work, we studied one-dimensional phononic structures for selective acoustic filtering. The structures are composed of three and four materials which have different elastic properties. We have observed that the phononic band gaps split in two and three transmission valleys for the three-material and the four-material based phononic structures, respectively. Furthermore, the number of transmission peaks between the split gaps is directly related to the number of unit cells composing the phononic structures. The observations of this work can be useful for the fabrication of acoustic filters with the possibility to select the transmission of particular frequencies.

  13. Engineering interactions between superconducting qubits and phononic nanostructures

    NASA Astrophysics Data System (ADS)

    Arrangoiz-Arriola, Patricio; Safavi-Naeini, Amir H.

    2016-12-01

    Nanomechanical systems can support highly coherent microwave-frequency excitations at cryogenic temperatures. However, generating sufficient coupling between these devices and superconducting quantum circuits is challenging due to the vastly different length scales of acoustic and electromagnetic excitations. Here we demonstrate a general method for calculating piezoelectric interactions between quantum circuits and arbitrary phononic nanostructures. We illustrate our technique by studying the coupling between a transmon qubit and bulk acoustic-wave, Lamb-wave, and phononic crystal resonators, and show that very large coupling rates are possible in all three cases. Our results suggest a route to phononic circuits and systems that are nonlinear at the single-phonon level.

  14. Anisotropic phonon coupling in the relaxor ferroelectric (Na1/2Bi1/2)TiO3 near its high-temperature phase transition

    NASA Astrophysics Data System (ADS)

    Cai, Ling; Toulouse, Jean; Luo, Haosu; Tian, Wei

    2014-08-01

    The lead free relaxor Na1/2Bi1/2TiO3 (NBT) undergoes a structural cubic-to-tetragonal transition near 800 K which is caused by the cooperative rotations of O6 octahedra. These rotations are also accompanied by the displacements of the cations and the formation of the polar nanodomains (PNDs) that are responsible for the characteristic dielectric dispersion of relaxor ferroelectrics. Because of their intrinsic properties, spontaneous polarization, and lack of inversion symmetry, these PNDs are also piezoelectric and can mediate an interaction between polarization and strain or couple the optic and acoustic phonons. Because PNDs introduce a local tetragonal symmetry, the phonon coupling they mediate is found to be anisotropic. In this paper we present inelastic neutron scattering results on coupled transverse acoustic (TA) and transverse optic (TO) phonons in the [110] and [001] directions and across the cubic-tetragonal phase transition at TC˜800 K. The phonon spectra are analyzed using a mode coupling model. In the [110] direction, as in other relaxors and some ferroelectric perovskites, a precipitous drop of the TO phonon into the TA branch or "waterfall" is observed at a certain qwf˜0.14 r.l.u. In the [001] direction, the highly overdamped line shape can be fitted with closely positioned bare mode energies which are largely overlapping along the dispersion curves. Two competing lattice coupling mechanism are proposed to explain these observations.

  15. Comment on "Attenuation and dispersion of sound in dilute suspensions of spherical particles" [J. Acoust. Soc. Am. 108(1), 126-146 (2000)].

    PubMed

    Shukla, Shiva Kant; Elvira, Luis

    2015-05-01

    Comment is made on an article by Temkin [J. Acoust. Soc. Am. 108(1), 126-146 (2000)]. This work illustrates the impact of particle size distribution on the dispersion and attenuation of sound waves propagating through particle suspensions. Temkin's propagation theory is extended for poly-disperse distributions of spherical particles, applicable to real suspensions. Significant changes in dispersion and attenuation appear near the particle resonance for both bubble and solid particle suspensions. Existing experimental data for bubble distributions also shows a good agreement with the poly-disperse modifications proposed.

  16. Dispersal

    USGS Publications Warehouse

    Clobert, J.; Danchin, E.; Dhondt, A.A.; Nichols, J.D.

    2001-01-01

    The ability of species to migrate and disperse is a trait that has interested ecologists for many years. Now that so many species and ecosystems face major environmental threats from habitat fragmentation and global climate change, the ability of species to adapt to these changes by dispersing, migrating, or moving between patches of habitat can be crucial to ensuring their survival. This book provides a timely and wide-ranging overview of the study of dispersal and incorporates much of the latest research. The causes, mechanisms, and consequences of dispersal at the individual, population, species and community levels are considered. The potential of new techniques and models for studying dispersal, drawn from molecular biology and demography, is also explored. Perspectives and insights are offered from the fields of evolution, conservation biology and genetics. Throughout the book, theoretical approaches are combined with empirical data, and care has been taken to include examples from as wide a range of species as possible.

  17. Band structures in two-dimensional phononic crystals with periodic Jerusalem cross slot

    NASA Astrophysics Data System (ADS)

    Li, Yinggang; Chen, Tianning; Wang, Xiaopeng; Yu, Kunpeng; Song, Ruifang

    2015-01-01

    In this paper, a novel two-dimensional phononic crystal composed of periodic Jerusalem cross slot in air matrix with a square lattice is presented. The dispersion relations and the transmission coefficient spectra are calculated by using the finite element method based on the Bloch theorem. The formation mechanisms of the band gaps are analyzed based on the acoustic mode analysis. Numerical results show that the proposed phononic crystal structure can yield large band gaps in the low-frequency range. The formation mechanism of opening the acoustic band gaps is mainly attributed to the resonance modes of the cavities inside the Jerusalem cross slot structure. Furthermore, the effects of the geometrical parameters on the band gaps are further explored numerically. Results show that the band gaps can be modulated in an extremely large frequency range by the geometry parameters such as the slot length and width. These properties of acoustic waves in the proposed phononic crystals can potentially be applied to optimize band gaps and generate low-frequency filters and waveguides.

  18. Non-equilibrium optical phonon dynamics in bulk and low-dimensional semiconductors

    NASA Astrophysics Data System (ADS)

    Srivastava, G. P.

    2007-02-01

    We present theoretical investigations of the intrinsic dynamics of long-wavelength non-equilibrium optical phonons in bulk and low-dimensional semiconductors. The theory is based on the application of Fermi's golden rule formula, with phonon dispersion relations as well as crystal anharmonicity considered in the framework of isotropic continuum model. Contributions to the decay rates of the phonon modes are discussed in terms of four possible channels: Klemens channel (into two acoustic daughter modes), generalised Ridley channel (into one acoustic and one optical mode), generalised Vallee-Bogani channel (into a lower mode of the same branch and an acoustic mode), and Barman-Srivastava channel (into two lower-branch optical modes). The role of crystal structure and cation/anion mass ratio in determining the lifetime of such modes in bulk semiconductors is highlighted. Estimates of lifetimes of such modes in silicon nanowires and carbon nanotubes will also be presented. The results support and explain available experimental data, and make predictions in some cases.

  19. Phonon manipulation with phononic crystals.

    SciTech Connect

    Kim Bongsang; Hopkins, Patrick Edward; Leseman, Zayd C.; Goettler, Drew F.; Su, Mehmet F.; El-Kady, Ihab Fathy; Reinke, Charles M.; Olsson, Roy H., III

    2012-01-01

    In this work, we demonstrated engineered modification of propagation of thermal phonons, i.e. at THz frequencies, using phononic crystals. This work combined theoretical work at Sandia National Laboratories, the University of New Mexico, the University of Colorado Boulder, and Carnegie Mellon University; the MESA fabrication facilities at Sandia; and the microfabrication facilities at UNM to produce world-leading control of phonon propagation in silicon at frequencies up to 3 THz. These efforts culminated in a dramatic reduction in the thermal conductivity of silicon using phononic crystals by a factor of almost 30 as compared with the bulk value, and about 6 as compared with an unpatterned slab of the same thickness. This work represents a revolutionary advance in the engineering of thermoelectric materials for optimal, high-ZT performance. We have demonstrated the significant reduction of the thermal conductivity of silicon using phononic crystal structuring using MEMS-compatible fabrication techniques and in a planar platform that is amenable to integration with typical microelectronic systems. The measured reduction in thermal conductivity as compared to bulk silicon was about a factor of 20 in the cross-plane direction [26], and a factor of 6 in the in-plane direction. Since the electrical conductivity was only reduced by a corresponding factor of about 3 due to the removal of conductive material (i.e., porosity), and the Seebeck coefficient should remain constant as an intrinsic material property, this corresponds to an effective enhancement in ZT by a factor of 2. Given the number of papers in literature devoted to only a small, incremental change in ZT, the ability to boost the ZT of a material by a factor of 2 simply by reducing thermal conductivity is groundbreaking. The results in this work were obtained using silicon, a material that has benefitted from enormous interest in the microelectronics industry and that has a fairly large thermoelectric power

  20. Flexocoupling impact on the generalized susceptibility and soft phonon modes in the ordered phase of ferroics

    SciTech Connect

    Morozovska, Anna N.; Vysochanskii, Yulian M.; Varenyk, Oleksandr V.; Silibin, Maxim V.; Kalinin, Sergei V.; Eliseev, Eugene A.

    2015-09-29

    The impact of the flexoelectric effect on the generalized susceptibility and soft phonon dispersion is not well known in the long-range-ordered phases of ferroics. Within the Landau-Ginzburg-Devonshire approach we obtained analytical expressions for the generalized susceptibility and phonon dispersion relations in the ferroelectric phase. The joint action of the static and dynamic flexoelectric effects induces nondiagonal components of the generalized susceptibility, whose amplitude is proportional to the convolution of the spontaneous polarization with the flexocoupling constants. The flexocoupling essentially broadens the k spectrum of the generalized susceptibility and leads to an additional “pushing away” of the optical and acoustic soft mode phonon branches. The degeneracy of the transverse optical and acoustic modes disappears in the ferroelectric phase in comparison with the paraelectric phase due to the joint action of flexoelectric coupling and ferroelectric nonlinearity. Lastly, the results obtained might be mainly important for theoretical analyses of a broad spectrum of experimental data, including neutron and Brillouin scattering.

  1. Flexocoupling impact on the generalized susceptibility and soft phonon modes in the ordered phase of ferroics

    DOE PAGES

    Morozovska, Anna N.; Vysochanskii, Yulian M.; Varenyk, Oleksandr V.; ...

    2015-09-29

    The impact of the flexoelectric effect on the generalized susceptibility and soft phonon dispersion is not well known in the long-range-ordered phases of ferroics. Within the Landau-Ginzburg-Devonshire approach we obtained analytical expressions for the generalized susceptibility and phonon dispersion relations in the ferroelectric phase. The joint action of the static and dynamic flexoelectric effects induces nondiagonal components of the generalized susceptibility, whose amplitude is proportional to the convolution of the spontaneous polarization with the flexocoupling constants. The flexocoupling essentially broadens the k spectrum of the generalized susceptibility and leads to an additional “pushing away” of the optical and acoustic softmore » mode phonon branches. The degeneracy of the transverse optical and acoustic modes disappears in the ferroelectric phase in comparison with the paraelectric phase due to the joint action of flexoelectric coupling and ferroelectric nonlinearity. Lastly, the results obtained might be mainly important for theoretical analyses of a broad spectrum of experimental data, including neutron and Brillouin scattering.« less

  2. Implementation of dispersion-free slow acoustic wave propagation and phase engineering with helical-structured metamaterials

    PubMed Central

    Zhu, Xuefeng; Li, Kun; Zhang, Peng; Zhu, Jie; Zhang, Jintao; Tian, Chao; Liu, Shengchun

    2016-01-01

    The ability to slow down wave propagation in materials has attracted significant research interest. A successful solution will give rise to manageable enhanced wave–matter interaction, freewheeling phase engineering and spatial compression of wave signals. The existing methods are typically associated with constructing dispersive materials or structures with local resonators, thus resulting in unavoidable distortion of waveforms. Here we show that, with helical-structured acoustic metamaterials, it is now possible to implement dispersion-free sound deceleration. The helical-structured metamaterials present a non-dispersive high effective refractive index that is tunable through adjusting the helicity of structures, while the wavefront revolution plays a dominant role in reducing the group velocity. Finally, we numerically and experimentally demonstrate that the helical-structured metamaterials with designed inhomogeneous unit cells can turn a normally incident plane wave into a self-accelerating beam on the prescribed parabolic trajectory. The helical-structured metamaterials will have profound impact to applications in explorations of slow wave physics. PMID:27198887

  3. Optic phonons and anisotropic thermal conductivity in hexagonal Ge2Sb2Te5

    PubMed Central

    Mukhopadhyay, Saikat; Lindsay, Lucas; Singh, David J.

    2016-01-01

    The lattice thermal conductivity (κ) of hexagonal Ge2Sb2Te5 (h-GST) is studied via direct first-principles calculations. We find significant intrinsic anisotropy (κa/κc~2) of κ in bulk h-GST, with the dominant contribution to κ from optic phonons, ~75%. This is extremely unusual as the acoustic phonon modes are the majority heat carriers in typical semiconductors and insulators. The anisotropy derives from varying bonding along different crystal directions, specifically from weak interlayer bonding along the c-axis, which gives anisotropic phonon dispersions. The phonon spectrum of h-GST has very dispersive optic branches with higher group velocities along the a-axis as compared to flat optic bands along the c-axis. The large optic mode contributions to the thermal conductivity in low-κ h-GST is unusual, and development of fundamental physical understanding of these contributions may be critical to better understanding of thermal conduction in other complex layered materials. PMID:27848985

  4. Optic phonons and anisotropic thermal conductivity in hexagonal Ge2Sb2Te5

    NASA Astrophysics Data System (ADS)

    Mukhopadhyay, Saikat; Lindsay, Lucas; Singh, David J.

    2016-11-01

    The lattice thermal conductivity (κ) of hexagonal Ge2Sb2Te5 (h-GST) is studied via direct first-principles calculations. We find significant intrinsic anisotropy (κa/κc~2) of κ in bulk h-GST, with the dominant contribution to κ from optic phonons, ~75%. This is extremely unusual as the acoustic phonon modes are the majority heat carriers in typical semiconductors and insulators. The anisotropy derives from varying bonding along different crystal directions, specifically from weak interlayer bonding along the c-axis, which gives anisotropic phonon dispersions. The phonon spectrum of h-GST has very dispersive optic branches with higher group velocities along the a-axis as compared to flat optic bands along the c-axis. The large optic mode contributions to the thermal conductivity in low-κ h-GST is unusual, and development of fundamental physical understanding of these contributions may be critical to better understanding of thermal conduction in other complex layered materials.

  5. Optic phonons and anisotropic thermal conductivity in hexagonal Ge2Sb2Te5

    DOE PAGES

    Mukhopadhyay, Saikat; Lindsay, Lucas R.; Singh, David

    2016-11-16

    The lattice thermal conductivity ($κ$) of hexagonal Ge2Sb2Tesub>5 (h-GST) is studied via direct first-principles calculations. We find significant intrinsic anisotropy of ( $κ$a/$κ$c~2) of $κ$ in bulk h-GST along different transport directions. The dominant contribution to$κ$ is from optic phonons, ~75%. This is extremely unusual as the acoustic phonon modes carry most of the heat in typical semiconductors and insulators with small unit cells. Very recently, Lee et. al. observed anisotropic in GST thin films and attributed this to thermal resistance of amorphous regions near grain boundaries. However, our results suggest an additional strong intrinsic anisotropy for the pure hexagonalmore » phase. This derives from bonding anisotropy along different crystal directions, specifically from weak interlayer coupling, which gives anisotropic phonon dispersions. The phonon spectrum of h-GST has very dispersive optic branches with higher group velocities along the a-axis as compared to flat optic bands along the c-axis. The importance of optic mode contributions for the thermal conductivity in low-$κ$ h-GST is unusual, and development of fundamental physical understanding of these contributions may be critical to better understanding of thermal conduction in other complex layered materials.« less

  6. Phonon impedance matching: minimizing interfacial thermal resistance of thin films

    NASA Astrophysics Data System (ADS)

    Polanco, Carlos; Zhang, Jingjie; Ghosh, Avik

    2014-03-01

    The challenge to minimize interfacial thermal resistance is to allow a broad band spectrum of phonons, with non-linear dispersion and well defined translational and rotational symmetries, to cross the interface. We explain how to minimize this resistance using a frequency dependent broadening matrix that generalizes the notion of acoustic impedance to the whole phonon spectrum including symmetries. We show how to ``match'' two given materials by joining them with a single atomic layer, with a multilayer material and with a graded superlattice. Atomic layer ``matching'' requires a layer with a mass close to the arithmetic mean (or spring constant close to the harmonic mean) to favor high frequency phonon transmission. For multilayer ``matching,'' we want a material with a broadening close to the geometric mean to maximize transmission peaks. For graded superlattices, a continuous sequence of geometric means translates to an exponentially varying broadening that generates a wide-band antireflection coating for both the coherent and incoherent limits. Our results are supported by ``first principles'' calculations of thermal conductance for GaAs / Gax Al1 - x As / AlAs thin films using the Non-Equilibrium Greens Function formalism coupled with Density Functional Perturbation Theory. NSF-CAREER (QMHP 1028883), NSF-IDR (CBET 1134311), XSEDE.

  7. Phonon spectral functions of photo-generated hot carrier plasmas: effects of carrier screening and plasmon-phonon coupling.

    PubMed

    Yi, Kyung-Soo; Kim, Hye-Jung

    2017-02-15

    We investigate spectral behavior of phonon spectral functions in an interacting multi-component hot carrier plasma. Spectral analysis of various phonon spectral functions is performed considering carrier-phonon channels of polar and nonpolar optical phonons, acoustic deformation-potential, and piezoelectric Coulomb couplings. Effects of phonon self-energy corrections are examined at finite temperature within a random phase approximation extended to include the effects of dynamic screening, plasmon-phonon coupling, and local-field corrections of the plasma species. We provide numerical data for the case of a photo-generated electron-hole plasma formed in a wurtzite GaN. Our result shows the clear significance of the multiplicity of the plasma species in the phonon spectral functions of a multi-component plasma giving rise to a variety of spectral behaviors of carrier-phonon coupled collective modes. A useful sum rule on the plasma-species-resolved dielectric functions is also found.

  8. Phonon spectral functions of photo-generated hot carrier plasmas: effects of carrier screening and plasmon-phonon coupling

    NASA Astrophysics Data System (ADS)

    Yi, Kyung-Soo; Kim, Hye-Jung

    2017-02-01

    We investigate spectral behavior of phonon spectral functions in an interacting multi-component hot carrier plasma. Spectral analysis of various phonon spectral functions is performed considering carrier-phonon channels of polar and nonpolar optical phonons, acoustic deformation-potential, and piezoelectric Coulomb couplings. Effects of phonon self-energy corrections are examined at finite temperature within a random phase approximation extended to include the effects of dynamic screening, plasmon-phonon coupling, and local-field corrections of the plasma species. We provide numerical data for the case of a photo-generated electron-hole plasma formed in a wurtzite GaN. Our result shows the clear significance of the multiplicity of the plasma species in the phonon spectral functions of a multi-component plasma giving rise to a variety of spectral behaviors of carrier-phonon coupled collective modes. A useful sum rule on the plasma-species-resolved dielectric functions is also found.

  9. Phononic crystals and elastodynamics: Some relevant points

    SciTech Connect

    Aravantinos-Zafiris, N.; Sigalas, M. M.; Kafesaki, M.; Economou, E. N.

    2014-12-15

    In the present paper we review briefly some of the first works on wave propagation in phononic crystals emphasizing the conditions for the creation of acoustic band-gaps and the role of resonances to the band-gap creation. We show that useful conclusions in the analysis of phononic band gap structures can be drawn by considering the mathematical similarities of the basic classical wave equation (Helmholtz equation) with Schrödinger equation and by employing basic solid state physics concepts and conclusions regarding electronic waves. In the second part of the paper we demonstrate the potential of phononic systems to be used as elastic metamaterials. This is done by demonstrating negative refraction in phononic crystals and subwavelength waveguiding in a linear chain of elastic inclusions, and by proposing a novel structure with close to pentamode behavior. Finally the potential of phononic structures to be used in liquid sensor applications is discussed and demonstrated.

  10. Phononic crystals and elastodynamics: Some relevant points

    NASA Astrophysics Data System (ADS)

    Aravantinos-Zafiris, N.; Sigalas, M. M.; Kafesaki, M.; Economou, E. N.

    2014-12-01

    In the present paper we review briefly some of the first works on wave propagation in phononic crystals emphasizing the conditions for the creation of acoustic band-gaps and the role of resonances to the band-gap creation. We show that useful conclusions in the analysis of phononic band gap structures can be drawn by considering the mathematical similarities of the basic classical wave equation (Helmholtz equation) with Schrödinger equation and by employing basic solid state physics concepts and conclusions regarding electronic waves. In the second part of the paper we demonstrate the potential of phononic systems to be used as elastic metamaterials. This is done by demonstrating negative refraction in phononic crystals and subwavelength waveguiding in a linear chain of elastic inclusions, and by proposing a novel structure with close to pentamode behavior. Finally the potential of phononic structures to be used in liquid sensor applications is discussed and demonstrated.

  11. Causality Bubbles to the Surface: Investigating Acoustic Causality in Highly Dispersive Bubbly Liquids

    DTIC Science & Technology

    2009-01-01

    media . This correction has resulted in a causal self-consistent theory verified by both higher fre- quency data taken in the Salt Water Tank Facility and...contemporary theories of acoustic propagation in bubbly media that has brought these theories into compliance with the physical law of causality. In...the experimental data below 10 kHz. FIGURE 2 Precision bubbler. This bubbler consists of 3000 luer-lock square cut hypodermic needles glued into a

  12. The Theory of Adaptive Dispersion and Acoustic-phonetic Properties of Cross-language Lexical-tone Systems

    NASA Astrophysics Data System (ADS)

    Alexander, Jennifer Alexandra

    Lexical-tone languages use fundamental frequency (F0/pitch) to convey word meaning. About 41.8% of the world's languages use lexical tone (Maddieson, 2008), yet those systems are under-studied. I aim to increase our understanding of speech-sound inventory organization by extending to tone-systems a model of vowel-system organization, the Theory of Adaptive Dispersion (TAD) (Liljencrants and Lindblom, 1972). This is a cross-language investigation of whether and how the size of a tonal inventory affects (A) acoustic tone-space size and (B) dispersion of tone categories within the tone-space. I compared five languages with very different tone inventories: Cantonese (3 contour, 3 level tones); Mandarin (3 contour, 1 level tone); Thai (2 contour, 3 level tones); Yoruba (3 level tones only); and Igbo (2 level tones only). Six native speakers (3 female) of each language produced 18 CV syllables in isolation, with each of his/her language's tones, six times. I measured tonal F0 across the vowel at onset, midpoint, and offglide. Tone-space size was the F0 difference in semitones (ST) between each language's highest and lowest tones. Tone dispersion was the F0 distance (ST) between two tones shared by multiple languages. Following the TAD, I predicted that languages with larger tone inventories would have larger tone-spaces. Against expectations, tone-space size was fixed across level-tone languages at midpoint and offglide, and across contour-tone languages (except Thai) at offglide. However, within each language type (level-tone vs. contour-tone), languages with smaller tone inventories had larger tone spaces at onset. Tone-dispersion results were also unexpected. The Cantonese mid-level tone was further dispersed from a tonal baseline than the Yoruba mid-level tone; Cantonese mid-level tone dispersion was therefore greater than theoretically necessary. The Cantonese high-level tone was also further dispersed from baseline than the Mandarin high-level tone -- at midpoint

  13. Variational derivation of the dispersion relation of kinetic coherent modes in the acoustic frequency range in tokamaks

    SciTech Connect

    Nguyen, C.; Garbet, X.; Smolyakov, A. I.

    2008-11-15

    In the present paper, we compare two modes with frequencies belonging to the acoustic frequency range: the geodesic acoustic mode (GAM) and the Beta Alfven eigenmode (BAE). For this, a variational gyrokinetic energy principle coupled to a Fourier sidebands expansion is developed. High order finite Larmor radius and finite orbit width effects are kept. Their impact on the mode structures and on the Alfven spectrum is calculated and discussed. We show that in a local analysis, the degeneracy of the electrostatic GAM and the BAE dispersion relations is verified to a high order and based in particular on a local poloidal symmetry of the two modes. When a more global point of view is taken, and the full radial structures of the modes are computed, differences appear. The BAE structure is shown to have an enforced localization, and to possibly connect to a large magnetohydrodynamic structure. On the contrary, the GAM is seen to have a wavelike, nonlocalized structure, as long as standard slowly varying monotonic profiles are considered.

  14. Measuring, interpreting, and translating electron quasiparticle - Phonon interactions on the surfaces of the topological insulators bismuth selenide and bismuth telluride

    NASA Astrophysics Data System (ADS)

    Howard, Colin

    The following dissertation presents a comprehensive study of the interaction between Dirac fermion quasiparticles (DFQs) and surface phonons on the surfaces of the topological insulators Bi2Se3 and Bi2Te 3. Inelastic helium atom surface scattering (HASS) spectroscopy and time of flight (TOF) techniques were used to measure the surface phonon dispersion of these materials along the two high-symmetry directions of the surface Brillouin zone (SBZ). Two anomalies common to both materials are exhibited in the experimental data. First, there is an absence of Rayleigh acoustic waves on the surface of these materials, pointing to weak coupling between the surface charge density and the surface acoustic phonon modes and potential applications for soundproofing technologies. Secondly, both materials exhibit an out-of-plane polarized optical phonon mode beginning at the SBZ center and dispersing to lower energy with increasing wave vector along both high-symmetry directions of the SBZ. This trend terminates in a V-shaped minimum at a wave vector corresponding to 2 kF for each material, after which the dispersion resumes its upward trend. This phenomenon constitutes a strong Kohn anomaly and can be attributed to the interaction between the surface phonons and DFQs. To quantify the coupling between the optical phonons experiencing strong renormalization and the DFQs at the surface, a phenomenological model was constructed based within the random phase approximation. Fitting the theoretical model to the experimental data allowed for the extraction of the matrix elements of the coupling Hamiltonian and the modifications to the surface phonon propagator encoded in the phonon self energy. This allowed, for the first time, calculation of phonon mode-specific quasiparticle-phonon coupling lambdanu( q) from experimental data. Additionally, an averaged coupling parameter was determined for both materials yielding bar lambdaTe ≈ 2 and bar lambdaSe ≈ 0.7. These values are

  15. Nonlinear acoustics in a dispersive continuum: Random waves, radiation pressure, and quantum noise

    NASA Astrophysics Data System (ADS)

    Cabot, M. A.

    The nonlinear interaction of sound with sound is studied using dispersive hydrodynamics which derived from a variational principle and the assumption that the internal energy density depends on gradients of the mass density. The attenuation of sound due to nonlinear interaction with a background is calculated and is shown to be sensitive to both the nature of the dispersion and decay bandwidths. The theoretical results are compared to those of low temperature helium experiments. A kinetic equation which described the nonlinear self-inter action of a background is derived. When a Deybe-type cutoff is imposed, a white noise distribution is shown to be a stationary distribution of the kinetic equation. The attenuation and spectrum of decay of a sound wave due to nonlinear interaction with zero point motion is calculated. In one dimension, the dispersive hydrodynamic equations are used to calculate the Langevin and Rayleigh radiation pressures of wave packets and solitary waves.

  16. Dispersion analysis and measurement of circular cylindrical wedge-like acoustic waveguides.

    PubMed

    Yu, Tai-Ho

    2015-09-01

    This study investigated the propagation of flexural waves along the outer edge of a circular cylindrical wedge, the phase velocities, and the corresponding mode displacements. Thus far, only approximate solutions have been derived because the corresponding boundary-value problems are complex. In this study, dispersion curves were determined using the bi-dimensional finite element method and derived through the separation of variables and the Hamilton principle. Modal displacement calculations clarified that the maximal deformations appeared at the outer edge of the wedge tip. Numerical examples indicated how distinct thin-film materials deposited on the outer surface of the circular cylindrical wedge influenced the dispersion curves. Additionally, dispersion curves were measured using a laser-induced guided wave, a knife-edge measurement scheme, and a two-dimensional fast Fourier transform method. Both the numerical and experimental results correlated closely, thus validating the numerical solution.

  17. Phonon dynamics of americium telluride

    NASA Astrophysics Data System (ADS)

    Arya, B. S.; Aynyas, Mahendra; Ahirwar, Ashok K.; Sanyal, S. P.

    2013-06-01

    We report for the first time the complete phonon dispersion curves for Americium telluride (AmTe) using a breathing shell models (BSM) to establish their predominant ionic nature. The results obtained in the present study show the general features of the phonon spectrum. We could not compare our results with the experimental measurements as they are not available so far. We emphasize the need of neutron scattering measurements to compare our results. We also report, for the first time specific heat for this compound.

  18. Phonons and elasticity of cementite through the Curie temperature

    NASA Astrophysics Data System (ADS)

    Mauger, L.; Herriman, J. E.; Hellman, O.; Tracy, S. J.; Lucas, M. S.; Muñoz, J. A.; Xiao, Yuming; Li, J.; Fultz, B.

    2017-01-01

    Phonon partial densities of states (pDOS) of Fe573C were measured from cryogenic temperatures through the Curie transition at 460 K using nuclear resonant inelastic x-ray scattering. The cementite pDOS reveal that low-energy acoustic phonons shift to higher energies (stiffen) with temperature before the magnetic transition. This unexpected stiffening suggests strongly nonharmonic vibrational behavior that impacts the thermodynamics and elastic properties of cementite. Density functional theory calculations reproduced the anomalous stiffening observed experimentally in cementite by accounting for phonon-phonon interactions at finite temperatures. The calculations show that the low-energy acoustic phonon branches with polarizations along the [010] direction are largely responsible for the anomalous thermal stiffening. The effect was further localized to the motions of the FeII site within the orthorhombic structure, which participates disproportionately in the anomalous phonon stiffening.

  19. Phononic crystal devices

    DOEpatents

    El-Kady, Ihab F [Albuquerque, NM; Olsson, Roy H [Albuquerque, NM

    2012-01-10

    Phononic crystals that have the ability to modify and control the thermal black body phonon distribution and the phonon component of heat transport in a solid. In particular, the thermal conductivity and heat capacity can be modified by altering the phonon density of states in a phononic crystal. The present invention is directed to phononic crystal devices and materials such as radio frequency (RF) tags powered from ambient heat, dielectrics with extremely low thermal conductivity, thermoelectric materials with a higher ratio of electrical-to-thermal conductivity, materials with phononically engineered heat capacity, phononic crystal waveguides that enable accelerated cooling, and a variety of low temperature application devices.

  20. Theoretical description based on general and exact nonextensive dispersion relations of plasma oscillation data and verification of new acoustic plasma waves

    SciTech Connect

    Ebrahimi, V.; Esfandyari-Kalejahi, A.

    2014-09-15

    In this paper, first we represent the differences between spatial and temporal dispersions and their dependence on the measurement techniques for electrostatic waves in unmagnetized collisionless plasma. Then, three different experimental data are compared to the solutions of exact nonextensive dispersion relations for electron-ion and pair plasma. The results confirm the existence of new acoustic plasma waves. Furthermore, these comparisons yield a Maxwellian and a nonextensive plasma with nonextensive parameter q larger than one, and a Maxwellian plasma with some abnormal dispersion properties.

  1. Audibility of dispersion error in room acoustic finite-difference time-domain simulation in the presence of absorption of air.

    PubMed

    Saarelma, Jukka; Savioja, Lauri

    2016-12-01

    The finite-difference time-domain method has gained increasing interest for room acoustic prediction use. A well-known limitation of the method is a frequency and direction dependent dispersion error. In this study, the audibility of dispersion error in the presence of air absorption is measured. The results indicate that the dispersion error in the worst-case direction of the studied scheme gets masked by the air absorption at a phase velocity error percentage of 0.28% at the frequency of 20 kHz.

  2. Determination of elastic properties of a MnO2 coating by surface acoustic wave velocity dispersion analysis

    NASA Astrophysics Data System (ADS)

    Sermeus, J.; Sinha, R.; Vanstreels, K.; Vereecken, P. M.; Glorieux, C.

    2014-07-01

    MnO2 is a material of interest in the development of high energy-density batteries, specifically as a coating material for internal 3D structures, thus ensuring rapid energy deployment. Its electrochemical properties have been mapped extensively, but there are, to the best of the authors' knowledge, no records of the elastic properties of thin film MnO2. Impulsive stimulated thermal scattering (ISTS), also known as the heterodyne diffraction or transient grating technique, was used to determine the Young's modulus (E) and porosity (ψ) of a 500 nm thick MnO2 coating on a Si(001) substrate. ISTS is an all optical method that is able to excite and detect surface acoustic waves (SAWs) on opaque samples. From the measured SAW velocity dispersion, the Young's modulus and porosity were determined to be E = 25 ± 1 GPa and ψ = 42 ± 1 %, respectively. These values were confirmed by independent techniques and determined by a most-squares analysis of the carefully fitted SAW velocity dispersion. This study demonstrates the ability of the presented technique to determine the elastic parameters of a thin, porous film on an anisotropic substrate.

  3. Atomistic modeling of phonon bandstructure and transport for optimal thermal management in nanoscale devices

    NASA Astrophysics Data System (ADS)

    Sundaresan, Sasi Sekaran

    Monte Carlo based statistical approach to solve Boltzmann Transport Equation (BTE) has become a norm to investigate heat transport in semiconductors at sub-micron regime, owing mainly to its ability to characterize realistically sized device geometries qualitatively. One of the primary issues with this technique is that the approach predominantly uses empirically fitted phonon dispersion relations as input to determine the properties of phonons so as to predict the thermal conductivity of specified material geometry. The empirically fitted dispersion relations assume harmonic approximation thereby failing to account for thermal expansion, interaction of lattice waves, effect of strain on spring stiffness, and accurate phonon-phonon interaction. To circumvent this problem, in this work, a coupled molecular mechanics-Monte Carlo (MM-MC) platform has been developed and used to solve the phonon Boltzmann Transport Equation (BTE) for the calculation of thermal conductivity of several novel and emerging nanostructures. The use of the quasi-anharmonic MM approach (as implemented in the open source NEMO 3-D software toolkit) not only allows one to capture the true atomicity of the underlying lattice but also enables the simulation of realistically-sized structures containing millions of atoms. As compared to the approach using an empirically fitted phonon dispersion relation, here, a 17% increase in the thermal conductivity for a silicon nanowire due to the incorporation of atomistic corrections in the LA (longitudinal acoustic) branch alone has been reported. The atomistically derived thermal conductivity as calculated from the MM-MC framework is then used in the modular design and analysis of (i) a silicon nanowire based thermoelectric cooler (TEC) unit, and (ii) a GaN/InN based nanostructured light emitting device (LED). It is demonstrated that the use of empirically fitted phonon bandstructure parameters overestimates the temperature difference between the hot and the

  4. Electron-phonon interactions from first principles

    NASA Astrophysics Data System (ADS)

    Giustino, Feliciano

    2017-01-01

    This article reviews the theory of electron-phonon interactions in solids from the point of view of ab initio calculations. While the electron-phonon interaction has been studied for almost a century, predictive nonempirical calculations have become feasible only during the past two decades. Today it is possible to calculate from first principles many materials properties related to the electron-phonon interaction, including the critical temperature of conventional superconductors, the carrier mobility in semiconductors, the temperature dependence of optical spectra in direct and indirect-gap semiconductors, the relaxation rates of photoexcited carriers, the electron mass renormalization in angle-resolved photoelectron spectra, and the nonadiabatic corrections to phonon dispersion relations. In this article a review of the theoretical and computational framework underlying modern electron-phonon calculations from first principles as well as landmark investigations of the electron-phonon interaction in real materials is given. The first part of the article summarizes the elementary theory of electron-phonon interactions and their calculations based on density-functional theory. The second part discusses a general field-theoretic formulation of the electron-phonon problem and establishes the connection with practical first-principles calculations. The third part reviews a number of recent investigations of electron-phonon interactions in the areas of vibrational spectroscopy, photoelectron spectroscopy, optical spectroscopy, transport, and superconductivity.

  5. Multiple Quantum Wells for P T -Symmetric Phononic Crystals

    NASA Astrophysics Data System (ADS)

    Poshakinskiy, A. V.; Poddubny, A. N.; Fainstein, A.

    2016-11-01

    We demonstrate that the parity-time symmetry for sound is realized in laser-pumped multiple-quantum-well structures. Breaking of the parity-time symmetry for the phonons with wave vectors corresponding to the Bragg condition makes the structure a highly selective acoustic wave amplifier. Single-mode distributed feedback phonon lasing is predicted for structures with realistic parameters.

  6. Net electron-phonon scattering rates in InN/GaN multiple quantum wells: The effects of an energy dependent acoustic deformation potential

    SciTech Connect

    Xia, H. Patterson, R.; Feng, Y.; Shrestha, S.; Conibeer, G.

    2014-08-11

    The rates of charge carrier relaxation by phonon emission are of substantial importance in the field of hot carrier solar cell, primarily in investigation of mechanisms to slow down hot carrier cooling. In this work, energy and momentum resolved deformation potentials relevant to electron-phonon scattering are computed for wurtzite InN and GaN as well as an InN/GaN multiple quantum well (MQW) superlattice using ab-initio methods. These deformation potentials reveal important features such as discontinuities across the electronic bandgap of the materials and variations over tens of eV. The energy dependence of the deformation potential is found to be very similar for wurtzite nitrides despite differences between the In and Ga pseudopotentials and their corresponding electronic band structures. Charge carrier relaxation by this mechanism is expected to be minimal for electrons within a few eV of the conduction band edge. However, hole scattering at energies more accessible to excitation by solar radiation is possible between heavy and light hole states. Moderate reductions in overall scattering rates are observed in MQW relative to the bulk nitride materials.

  7. Phonons in active microfluidic crystals

    NASA Astrophysics Data System (ADS)

    Tsang, Alan Cheng Hou; Kanso, Eva

    2016-11-01

    One-dimensional crystals of driven particles confined in quasi two-dimensional microfluidic channels have been shown to exhibit propagating sound waves in the form of 'phonons', including both transverse and longitudinal normal modes. Here, we focus on one-dimensional crystals of motile particles in uniform external flows. We study the propagation of phonons in the context of an idealized model that accounts for hydrodynamic interactions among the motile particles. We obtain a closed-form analytical expression for the dispersion relation of the phonons. In the moving frame of reference of the crystals, the traveling directions of the phonons depend on the intensity of the external flow, and are exactly opposite for the transverse and longitudinal modes. We further investigate the stability of the phonons and show that the longitudinal mode is linearly stable, whereas the transverse mode is subject to an instability arising from the activity and orientation dynamics of the motile particles. These findings are important for understanding the propagation of disturbances and instabilities in confined motile particles, and could generate practical insights into the transport of motile cells in microfluidic devices.

  8. Acoustic Attenuation Probe for Fermion Superfluidity in Ultracold-Atom Gases

    SciTech Connect

    Gaudio, Sergio; Mihaila, Bogdan; Blagoev, Krastan B.; Timmermans, Eddy; Bedell, Kevin S.

    2007-03-16

    Dilute gas Bose-Einstein condensates (BEC's), currently used to cool fermionic atoms in atom traps, can also probe the superfluidity of these fermions. The damping rate of BEC-acoustic excitations (phonon modes), measured in the middle of the trap as a function of the phonon momentum, yields an unambiguous signature of BCS-like superfluidity, provides a measurement of the superfluid gap parameter, and gives an estimate of the size of the Cooper pairs in the BEC-BCS crossover regime. We also predict kinks in the momentum dependence of the damping rate which can reveal detailed information about the fermion quasiparticle dispersion relation.

  9. A dispersion relation in bidust acoustic wave in non uniform stratified plasma

    SciTech Connect

    Valdeblanquez, E.

    2006-12-04

    Low frequencies waves are studied in plasma with two kind of dusty grains. Also considered are stratified plasma with layers of different densities to that of the main plasma. In this analysis each dust species is treated with a simplified model of fluid equations, and electrons and ions are determined by a Boltzmann factor. Relative velocities between each species and the non uniform plasma is considered in order to study instabilities. In cases in which the speed or the density of current of the charged dust grains is zero, the dispersion equation is recovered.

  10. Nonlinear acoustic pulse propagation in dispersive sediments using fractional loss operators.

    PubMed

    Maestas, Joseph T; Collis, Jon M

    2016-03-01

    The nonlinear progressive wave equation (NPE) is a time-domain formulation of the Euler fluid equations designed to model low-angle wave propagation using a wave-following computational domain. The wave-following frame of reference permits the simulation of long-range propagation and is useful in modeling blast wave effects in the ocean waveguide. Existing models do not take into account frequency-dependent sediment attenuation, a feature necessary for accurately describing sound propagation over, into, and out of the ocean sediment. Sediment attenuation is addressed in this work by applying lossy operators to the governing equation that are based on a fractional Laplacian. These operators accurately describe frequency-dependent attenuation and dispersion in typical ocean sediments. However, dispersion within the sediment is found to be a secondary process to absorption and effectively negligible for ranges of interest. The resulting fractional NPE is benchmarked against a Fourier-transformed parabolic equation solution for a linear case, and against the analytical Mendousse solution to Burgers' equation for the nonlinear case. The fractional NPE is then used to investigate the effects of attenuation on shock wave propagation.

  11. Thermal transport and anharmonic phonons in strained monolayer hexagonal boron nitride

    PubMed Central

    Li, Shasha; Chen, Yue

    2017-01-01

    Thermal transport and phonon-phonon coupling in monolayer hexagonal boron nitride (h-BN) under equibiaxial strains are investigated from first principles. Phonon spectra at elevated temperatures have been calculated from perturbation theory using the third-order anharmonic force constants. The stiffening of the out-of-plane transverse acoustic mode (ZA) near the Brillouin zone center and the increase of acoustic phonon lifetimes are found to contribute to the dramatic increase of thermal transport in strained h-BN. The transverse optical mode (TO) at the K point, which was predicted to lead to mechanical failure of h-BN, is found to shift to lower frequencies at elevated temperatures under equibiaxial strains. The longitudinal and transverse acoustic modes exhibit broad phonon spectra under large strains in sharp contrast to the ZA mode, indicating strong in-plane phonon-phonon coupling. PMID:28262786

  12. Thermal transport and anharmonic phonons in strained monolayer hexagonal boron nitride.

    PubMed

    Li, Shasha; Chen, Yue

    2017-03-06

    Thermal transport and phonon-phonon coupling in monolayer hexagonal boron nitride (h-BN) under equibiaxial strains are investigated from first principles. Phonon spectra at elevated temperatures have been calculated from perturbation theory using the third-order anharmonic force constants. The stiffening of the out-of-plane transverse acoustic mode (ZA) near the Brillouin zone center and the increase of acoustic phonon lifetimes are found to contribute to the dramatic increase of thermal transport in strained h-BN. The transverse optical mode (TO) at the K point, which was predicted to lead to mechanical failure of h-BN, is found to shift to lower frequencies at elevated temperatures under equibiaxial strains. The longitudinal and transverse acoustic modes exhibit broad phonon spectra under large strains in sharp contrast to the ZA mode, indicating strong in-plane phonon-phonon coupling.

  13. Thermal transport and anharmonic phonons in strained monolayer hexagonal boron nitride

    NASA Astrophysics Data System (ADS)

    Li, Shasha; Chen, Yue

    2017-03-01

    Thermal transport and phonon-phonon coupling in monolayer hexagonal boron nitride (h-BN) under equibiaxial strains are investigated from first principles. Phonon spectra at elevated temperatures have been calculated from perturbation theory using the third-order anharmonic force constants. The stiffening of the out-of-plane transverse acoustic mode (ZA) near the Brillouin zone center and the increase of acoustic phonon lifetimes are found to contribute to the dramatic increase of thermal transport in strained h-BN. The transverse optical mode (TO) at the K point, which was predicted to lead to mechanical failure of h-BN, is found to shift to lower frequencies at elevated temperatures under equibiaxial strains. The longitudinal and transverse acoustic modes exhibit broad phonon spectra under large strains in sharp contrast to the ZA mode, indicating strong in-plane phonon-phonon coupling.

  14. Enhancing phonon flow through one-dimensional interfaces by impedance matching

    SciTech Connect

    Polanco, Carlos A. Ghosh, Avik W.

    2014-08-28

    We extend concepts from microwave engineering to thermal interfaces and explore the principles of impedance matching in 1D. The extension is based on the generalization of acoustic impedance to nonlinear dispersions using the contact broadening matrix Γ(ω), extracted from the phonon self energy. For a single junction, we find that for coherent and incoherent phonons, the optimal thermal conductance occurs when the matching Γ(ω) equals the Geometric Mean of the contact broadenings. This criterion favors the transmission of both low and high frequency phonons by requiring that (1) the low frequency acoustic impedance of the junction matches that of the two contacts by minimizing the sum of interfacial resistances and (2) the cut-off frequency is near the minimum of the two contacts, thereby reducing the spillage of the states into the tunneling regime. For an ultimately scaled single atom/spring junction, the matching criterion transforms to the arithmetic mean for mass and the harmonic mean for spring constant. The matching can be further improved using a composite graded junction with an exponential varying broadening that functions like a broadband antireflection coating. There is, however, a trade off as the increased length of the interface brings in additional intrinsic sources of scattering.

  15. Phonon triggered rhombohedral lattice distortion in vanadium at high pressure

    SciTech Connect

    Antonangeli, Daniele; Farber, Daniel L.; Bosak, Alexei; Aracne, Chantel M.; Ruddle, David G.; Krisch, Michael

    2016-08-19

    In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Lastly, our results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V.

  16. Phonon triggered rhombohedral lattice distortion in vanadium at high pressure.

    PubMed

    Antonangeli, Daniele; Farber, Daniel L; Bosak, Alexei; Aracne, Chantel M; Ruddle, David G; Krisch, Michael

    2016-08-19

    In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Our results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V.

  17. Phonon triggered rhombohedral lattice distortion in vanadium at high pressure

    DOE PAGES

    Antonangeli, Daniele; Farber, Daniel L.; Bosak, Alexei; ...

    2016-08-19

    In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Lastly, ourmore » results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V.« less

  18. Phonon triggered rhombohedral lattice distortion in vanadium at high pressure

    PubMed Central

    Antonangeli, Daniele; Farber, Daniel L.; Bosak, Alexei; Aracne, Chantel M.; Ruddle, David G.; Krisch, Michael

    2016-01-01

    In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Our results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V. PMID:27539662

  19. Revealing the mechanism of passive transport in lipid bilayers via phonon-mediated nanometre-scale density fluctuations

    SciTech Connect

    Zhernenkov, Mikhail; Bolmatov, Dima; Soloviov, Dmitry; Zhernenkov, Kirill; Toperverg, Boris P.; Cunsolo, Alessandro; Bosak, Alexey; Cai, Yong

    2016-05-12

    We report the high resolution inelastic x-ray study of the in-plane phonon excitations in dipalmitoyl phosphatidylcholine (DPPC) above and below main transition temperature. In the Lβ' gel phase, we observe high frequency longitudinal phonon mode previously predicted by the molecular dynamics simulations and for the first time, we reveal low frequency weakly dispersive transverse acoustic mode which softens and exhibits a low-frequency phonon gap when the DPPC lipid transitions into the Lα fluid phase. The phonon softening of the high frequency longitudinal excitations and the transformation of the transverse excitations upon the phase transition from the Lβ' to Lα phase is explained within the framework of the phonon theory of liquids. These findings illustrate the importance of the collective dynamics of biomembranes and reveal that hydrocarbon tails can act as an efficient mediator in controlling the passive transport across the bilayer plane.

  20. Modeling power law absorption and dispersion for acoustic propagation using the fractional Laplacian.

    PubMed

    Treeby, Bradley E; Cox, B T

    2010-05-01

    The efficient simulation of wave propagation through lossy media in which the absorption follows a frequency power law has many important applications in biomedical ultrasonics. Previous wave equations which use time-domain fractional operators require the storage of the complete pressure field at previous time steps (such operators are convolution based). This makes them unsuitable for many three-dimensional problems of interest. Here, a wave equation that utilizes two lossy derivative operators based on the fractional Laplacian is derived. These operators account separately for the required power law absorption and dispersion and can be efficiently incorporated into Fourier based pseudospectral and k-space methods without the increase in memory required by their time-domain fractional counterparts. A framework for encoding the developed wave equation using three coupled first-order constitutive equations is discussed, and the model is demonstrated through several one-, two-, and three-dimensional simulations.

  1. Two-Dimensional Phononic Crystals: Disorder Matters.

    PubMed

    Wagner, Markus R; Graczykowski, Bartlomiej; Reparaz, Juan Sebastian; El Sachat, Alexandros; Sledzinska, Marianna; Alzina, Francesc; Sotomayor Torres, Clivia M

    2016-09-14

    The design and fabrication of phononic crystals (PnCs) hold the key to control the propagation of heat and sound at the nanoscale. However, there is a lack of experimental studies addressing the impact of order/disorder on the phononic properties of PnCs. Here, we present a comparative investigation of the influence of disorder on the hypersonic and thermal properties of two-dimensional PnCs. PnCs of ordered and disordered lattices are fabricated of circular holes with equal filling fractions in free-standing Si membranes. Ultrafast pump and probe spectroscopy (asynchronous optical sampling) and Raman thermometry based on a novel two-laser approach are used to study the phononic properties in the gigahertz (GHz) and terahertz (THz) regime, respectively. Finite element method simulations of the phonon dispersion relation and three-dimensional displacement fields furthermore enable the unique identification of the different hypersonic vibrations. The increase of surface roughness and the introduction of short-range disorder are shown to modify the phonon dispersion and phonon coherence in the hypersonic (GHz) range without affecting the room-temperature thermal conductivity. On the basis of these findings, we suggest a criteria for predicting phonon coherence as a function of roughness and disorder.

  2. Toward stimulated interaction of surface phonon polaritons

    SciTech Connect

    Kong, B. D.; Trew, R. J.; Kim, K. W.

    2013-12-21

    Thermal emission spectra mediated by surface phonon polariton are examined by using a theoretical model that accounts for generation processes. Specifically, the acoustic phonon fusion mechanism is introduced to remedy theoretical deficiencies of the near thermal equilibrium treatments. The model clarifies the thermal excitation mechanism of surface phonon polaritons and the energy transfer path under non-zero energy flow. When applied to GaAs and SiC semi-infinite surfaces, the nonequilibrium model predicts that the temperature dependence of the quasi-monochromatic peak can exhibit distinctly different characteristics of either sharp increase or slow saturation depending on the materials, which is in direct contrast with the estimate made by the near-equilibrium model. The proposed theoretical tool can accurately analyze the nonequilibrium steady states, potentially paving a pathway to demonstrate stimulated interaction/emission of thermally excited surface phonon polaritons.

  3. Toward stimulated interaction of surface phonon polaritons

    NASA Astrophysics Data System (ADS)

    Kong, B. D.; Trew, R. J.; Kim, K. W.

    2013-12-01

    Thermal emission spectra mediated by surface phonon polariton are examined by using a theoretical model that accounts for generation processes. Specifically, the acoustic phonon fusion mechanism is introduced to remedy theoretical deficiencies of the near thermal equilibrium treatments. The model clarifies the thermal excitation mechanism of surface phonon polaritons and the energy transfer path under non-zero energy flow. When applied to GaAs and SiC semi-infinite surfaces, the nonequilibrium model predicts that the temperature dependence of the quasi-monochromatic peak can exhibit distinctly different characteristics of either sharp increase or slow saturation depending on the materials, which is in direct contrast with the estimate made by the near-equilibrium model. The proposed theoretical tool can accurately analyze the nonequilibrium steady states, potentially paving a pathway to demonstrate stimulated interaction/emission of thermally excited surface phonon polaritons.

  4. Visco-elastic effects on wave dispersion in three-phase acoustic metamaterials

    NASA Astrophysics Data System (ADS)

    Krushynska, A. O.; Kouznetsova, V. G.; Geers, M. G. D.

    2016-11-01

    This paper studies the wave attenuation performance of dissipative solid acoustic metamaterials (AMMs) with local resonators possessing subwavelength band gaps. The metamaterial is composed of dense rubber-coated inclusions of a circular shape embedded periodically in a matrix medium. Visco-elastic material losses present in a matrix and/or resonator coating are introduced by either the Kelvin-Voigt or generalized Maxwell models. Numerical solutions are obtained in the frequency domain by means of k(ω)-approach combined with the finite element method. Spatially attenuating waves are described by real frequencies ω and complex-valued wave vectors k. Complete 3D band structure diagrams including complex-valued pass bands are evaluated for the undamped linear elastic and several visco-elastic AMM cases. The changes in the band diagrams due to the visco-elasticity are discussed in detail; the comparison between the two visco-elastic models representing artificial (Kelvin-Voigt model) and experimentally characterized (generalized Maxwell model) damping is performed. The interpretation of the results is facilitated by using attenuation and transmission spectra. Two mechanisms of the energy absorption, i.e. due to the resonance of the inclusions and dissipative effects in the materials, are discussed separately. It is found that the visco-elastic damping of the matrix material decreases the attenuation performance of AMMs within band gaps; however, if the matrix material is slightly damped, it can be modeled as linear elastic without the loss of accuracy given the resonator coating is dissipative. This study also demonstrates that visco-elastic losses properly introduced in the resonator coating improve the attenuation bandwidth of AMMs although the attenuation on the resonance peaks is reduced.

  5. Harnessing fluid-structure interactions to design self-regulating acoustic metamaterials

    NASA Astrophysics Data System (ADS)

    Casadei, Filippo; Bertoldi, Katia

    2014-01-01

    The design of phononic crystals and acoustic metamaterials with tunable and adaptive wave properties remains one of the outstanding challenges for the development of next generation acoustic devices. We report on the numerical and experimental demonstration of a locally resonant acoustic metamaterial with dispersion characteristics, which autonomously adapt in response to changes of an incident aerodynamic flow. The metamaterial consists of a slender beam featuring a periodic array or airfoil-shaped masses supported by a linear and torsional springs. The resonance characteristics of the airfoils lead to strong attenuation at frequencies defined by the properties of the airfoils and the speed on the incident fluid. The proposed concept expands the ability of existing acoustic bandgap materials to autonomously adapt their dispersion properties through fluid-structure interactions, and has the potential to dramatically impact a variety of applications, such as robotics, civil infrastructures, and defense systems.

  6. Harnessing fluid-structure interactions to design self-regulating acoustic metamaterials

    SciTech Connect

    Casadei, Filippo; Bertoldi, Katia

    2014-01-21

    The design of phononic crystals and acoustic metamaterials with tunable and adaptive wave properties remains one of the outstanding challenges for the development of next generation acoustic devices. We report on the numerical and experimental demonstration of a locally resonant acoustic metamaterial with dispersion characteristics, which autonomously adapt in response to changes of an incident aerodynamic flow. The metamaterial consists of a slender beam featuring a periodic array or airfoil-shaped masses supported by a linear and torsional springs. The resonance characteristics of the airfoils lead to strong attenuation at frequencies defined by the properties of the airfoils and the speed on the incident fluid. The proposed concept expands the ability of existing acoustic bandgap materials to autonomously adapt their dispersion properties through fluid-structure interactions, and has the potential to dramatically impact a variety of applications, such as robotics, civil infrastructures, and defense systems.

  7. Weak coupling of pseudoacoustic phonons and magnon dynamics in the incommensurate spin-ladder compound S r14C u24O41

    NASA Astrophysics Data System (ADS)

    Chen, Xi; Bansal, Dipanshu; Sullivan, Sean; Abernathy, Douglas L.; Aczel, Adam A.; Zhou, Jianshi; Delaire, Olivier; Shi, Li

    2016-10-01

    Intriguing lattice dynamics have been predicted for aperiodic crystals that contain incommensurate substructures. Here we report inelastic neutron scattering measurements of phonon and magnon dispersions in S r14C u24O41 , which contains incommensurate one-dimensional (1D) chain and two-dimensional (2D) ladder substructures. Two distinct pseudoacoustic phonon modes, corresponding to the sliding motion of one sublattice against the other, are observed for atomic motions polarized along the incommensurate axis. In the long wavelength limit, it is found that the sliding mode shows a remarkably small energy gap of 1.7-1.9 meV, indicating very weak interactions between the two incommensurate sublattices. The measurements also reveal a gapped and steep linear magnon dispersion of the ladder sublattice. The high group velocity of this magnon branch and weak coupling with acoustic and pseudoacoustic phonons can explain the large magnon thermal conductivity in S r14C u24O41 crystals. In addition, the magnon specific heat is determined from the measured total specific heat and phonon density of states and exhibits a Schottky anomaly due to gapped magnon modes of the spin chains. These findings offer new insights into the phonon and magnon dynamics and thermal transport properties of incommensurate magnetic crystals that contain low-dimensional substructures.

  8. Weak coupling of pseudoacoustic phonons and magnon dynamics in the incommensurate spin-ladder compound Sr14Cu24O41

    DOE PAGES

    Chen, Xi; Bansal, Dipanshu; Sullivan, Sean; ...

    2016-10-21

    Intriguing lattice dynamics have been predicted for aperiodic crystals that contain incommensurate substructures. Here we report inelastic neutron scattering measurements of phonon and magnon dispersions in Sr14Cu24O41, which contains incommensurate one-dimensional (1D) chain and two-dimensional (2D) ladder substructures. Two distinct pseudoacoustic phonon modes, corresponding to the sliding motion of one sublattice against the other, are observed for atomic motions polarized along the incommensurate axis. In the long wavelength limit, it is found that the sliding mode shows a remarkably small energy gap of 1.7–1.9 meV, indicating very weak interactions between the two incommensurate sublattices. The measurements also reveal a gappedmore » and steep linear magnon dispersion of the ladder sublattice. The high group velocity of this magnon branch and weak coupling with acoustic and pseudoacoustic phonons can explain the large magnon thermal conductivity in Sr14Cu24O41 crystals. In addition, the magnon specific heat is determined from the measured total specific heat and phonon density of states and exhibits a Schottky anomaly due to gapped magnon modes of the spin chains. Furthermore, these findings offer new insights into the phonon and magnon dynamics and thermal transport properties of incommensurate magnetic crystals that contain low-dimensional substructures.« less

  9. Predicting absorption and dispersion in acoustics by direct simulation Monte Carlo: Quantum and classical models for molecular relaxation.

    PubMed

    Hanford, Amanda D; O'Connor, Patrick D; Anderson, James B; Long, Lyle N

    2008-06-01

    In the current study, real gas effects in the propagation of sound waves are simulated using the direct simulation Monte Carlo method for a wide range of frequencies. This particle method allows for treatment of acoustic phenomena at high Knudsen numbers, corresponding to low densities and a high ratio of the molecular mean free path to wavelength. Different methods to model the internal degrees of freedom of diatomic molecules and the exchange of translational, rotational and vibrational energies in collisions are employed in the current simulations of a diatomic gas. One of these methods is the fully classical rigid-rotor/harmonic-oscillator model for rotation and vibration. A second method takes into account the discrete quantum energy levels for vibration with the closely spaced rotational levels classically treated. This method gives a more realistic representation of the internal structure of diatomic and polyatomic molecules. Applications of these methods are investigated in diatomic nitrogen gas in order to study the propagation of sound and its attenuation and dispersion along with their dependence on temperature. With the direct simulation method, significant deviations from continuum predictions are also observed for high Knudsen number flows.

  10. Phononic Origins of Friction in Carbon Nanotube Oscillators.

    PubMed

    Prasad, Matukumilli V D; Bhattacharya, Baidurya

    2017-03-01

    Phononic coupling can have a significant role in friction between nanoscale surfaces. We find frictional dissipation per atom in carbon nanotube (CNT) oscillators to depend significantly on interface features such as contact area, commensurability, and by end-capping of the inner core. We perform large-scale phonon wavepacket MD simulations to study phonon coupling between a 250 nm long (10,10) outer tube and inner cores of four different geometries. Five different phonon polarizations known to have dominant roles in thermal transport are selected, and transmission coefficient plots for a range of phonon energies along with phonon scattering dynamics at specific energies are obtained. We find that the length of interface affects friction only through LA phonon scattering and has a significant nonlinear effect on total frictional force. Incommensurate contact does not always give rise to superlubricity: the net effect of two competing interaction mechanisms shown by longitudinal and transverse phonons decides the role of commensurability. Capping of the core has no effect on acoustic phonons but destroys the coherence of transverse optical phonons and creates diffusive scattering. In contrast, the twisting and radial breathing phonon modes have perfect transmission at all energies and can be deemed as the enablers of ultralow friction in CNT oscillators. Our work suggests that tuning of interface geometries can give rise to desirable friction properties in nanoscale devices.

  11. Investigation of dispersion-relation-preserving scheme and spectral analysis methods for acoustic waves

    NASA Technical Reports Server (NTRS)

    Vanel, Florence O.; Baysal, Oktay

    1995-01-01

    Important characteristics of the aeroacoustic wave propagation are mostly encoded in their dispersion relations. Hence, a computational aeroacoustic (CAA) algorithm, which reasonably preserves these relations, was investigated. It was derived using an optimization procedure to ensure, that the numerical derivatives preserved the wave number and angular frequency of the differential terms in the linearized, 2-D Euler equations. Then, simulations were performed to validate the scheme and a compatible set of discretized boundary conditions. The computational results were found to agree favorably with the exact solutions. The boundary conditions were transparent to the outgoing waves, except when the disturbance source was close to a boundary. The time-domain data generated by such CAA solutions were often intractable until their spectra was analyzed. Therefore, the relative merits of three different methods were included in the study. For simple, periodic waves, the periodogram method produced better estimates of the steep-sloped spectra than the Blackman-Tukey method. Also, for this problem, the Hanning window was more effective when used with the weighted-overlapped-segment-averaging and Blackman-Tukey methods gave better results than the periodogram method. Finally, it was demonstrated that the representation of time domain-data was significantly dependent on the particular spectral analysis method employed.

  12. Acoustic scattering in dispersions: improvements in the calculation of single particle scattering coefficients.

    PubMed

    Pinfield, Valerie J

    2007-07-01

    Measurements of ultrasound speed and attenuation can be related to the properties of dispersed systems by applying a scattering model. Rayleigh's method for scattering of sound by a spherical object, and its subsequent developments to include viscous, thermal, and other effects (known as the ECAH model) has been widely adopted. The ECAH method has difficulties, including numerical ill-conditioning, calculation of Bessel functions at large arguments, and inclusion of thermal effects in all cases. The present work develops techniques for improving the ECAH calculations to allow its use in instrumentation. It is shown that thermal terms can be neglected in some boundary equations up to approximately 100 GHz in water, and several simplified solutions result. An analytical solution for the zero-order coefficient is presented, with separate nonthermal and thermal parts, allowing estimation of the thermal contribution. Higher orders have been simplified by estimating the small shear contribution as the inertial limit is approached. The condition of the matrix solutions have been greatly improved by these techniques and by including appropriate scaling factors. A method is presented for calculating the required Bessel functions when the argument is large (high frequency or large particle size). The required number of partial wave orders is also considered.

  13. Control of elastic wave propagation in one-dimensional piezomagnetic phononic crystals.

    PubMed

    Ponge, Marie-Fraise; Croënne, Charles; Vasseur, Jérôme O; Bou Matar, Olivier; Hladky-Hennion, Anne-Christine; Dubus, Bertrand

    2016-06-01

    Two ways of controlling the acoustic waves propagation by external inductance or capacitance in a one-dimensional (1-D) piezomagnetic phononic crystal are investigated. The structure is made of identical bars, constituted of a piezomagnetic material, surrounded by a coil and connected to an external impedance. A model of propagation of longitudinal elastic waves through the periodic structure is developed and the dispersion equation is obtained. Reflection and transmission coefficients are derived from a 2 × 2 transfer matrix formalism that also allows for the calculation of elastic effective parameters (density, Young modulus, speed of sound, impedance). The effect of shunting impedances is numerically investigated. The results reveal that a connected external inductance tunes the Bragg band gaps of the 1-D phononic crystal. When the elements are connected via a capacitance, a hybridization gap, due to the resonance of the LC circuit made of the piezomagnetic element and the capacitance, coexists with the Bragg band gap. The value of the external capacitance modifies the boundaries of both gaps. Calculation of the effective characteristics of the phononic crystal leads to an analysis of the physical mechanisms involved in the wave propagation. When periodically connected to external capacitances, a homogeneous piezomagnetic stack behaves as a dispersive tunable metamaterial.

  14. Renormalisation of Nonequilibrium Phonons Under Strong Perturbative Influences.

    NASA Astrophysics Data System (ADS)

    Mehta, Sushrut Madhukar

    Effects of strong perturbative influences, namely the presence of a narrow distribution of acoustic phonons, and the presence of an electron plasma, on the dynamics of nonequilibrium, near zone center, longitudinal optical phonons in GaP have been investigated in two separate experiments. The study of the effects of the interaction between the LO phonons and a heavily populated, narrow distribution of acoustic phonons lead to the observation of a new optically driven nonequilibrium phonon state. Time Resolved Coherent Antistokes Raman Scattering (TR-CARS), with picosecond resolution, was used to investigate the new mode. In order to achieve high occupation numbers in the acoustic branch, the picosecond laser pulses used were amplified up to 1.0 GW/cm^2 peak power per laser beam. An important characteristic property of the new state which differentiates it from the well known LO phonon state is the fact that rather than having the single decay rate observed under thermal equilibrium, the new state has two decay rates. Moreover, these two decay rates depend strongly on the distribution of the acoustic phonon occupation number. The coupling of the LO phonons with an electron plasma, on the other hand, was investigated by measurements of the shape of the Raman scattered line associated with the phonon-plasmon coupled mode. The plasma was generated by thermal excitation of carriers in doped samples. It was possible to study a large variety of plasma excitations by controlling the concentration of the dopant and the ambient temperature. A complete, self consistant model based on standard dielectric response theory is presented, and applied to the measurements of the phonon-plasmon coupled mode. It is possible to recover, via this model, the effective coupled mode damping rate, the plasma damping rate, and the plasma frequency as functions of ambient temperature, or the carrier concentration.

  15. Manipulation of Phonons with Phononic Crystals

    SciTech Connect

    Leseman, Zayd Chad

    2015-07-09

    There were three research goals associated with this project. First, was to experimentally demonstrate phonon spectrum control at THz frequencies using Phononic Crystals (PnCs), i.e. demonstrate coherent phonon scattering with PnCs. Second, was to experimentally demonstrate analog PnC circuitry components at GHz frequencies. The final research goal was to gain a fundamental understanding of phonon interaction using computational methods. As a result of this work, 7 journal papers have been published, 1 patent awarded, 14 conference presentations given, 4 conference publications, and 2 poster presentations given.

  16. Interaction of excitons with optical phonons in layer crystals

    NASA Astrophysics Data System (ADS)

    Nitsovich, Bohdan M.; Zenkova, C. Y.; Kramar, N. K.

    2002-02-01

    The investigation is concerned with layer crystals of the GaSe, InSe, GaTe, MoS2-type and other inorganic semiconductors, whose phonon spectrum has a great number of peculiarities, among them the availability of low-energy optical phonons. In this case the dispersion of these phonons can be essential and vary in character. The mass operator of the exciton-phonon system and the light absorption coefficient for different dispersion laws of optical phonons have been calculated. The influence of the sign of the phonon 'effective mass' on the exciton absorption band of layer crystals, which causes the opposite in sign dynamics of the absorption maximum shift, and the change of the absorption curve asymmetry have been determined.

  17. Phonon Scattering Dynamics of Thermophoretic Motion in Carbon Nanotube Oscillators.

    PubMed

    Prasad, Matukumilli V D; Bhattacharya, Baidurya

    2016-04-13

    Using phonon wave packet molecular dynamics simulations, we find that anomalous longitudinal acoustic (LA) mode phonon scattering in low to moderate energy ranges is responsible for initiating thermophoretic motion in carbon nanotube oscillators. The repeated scattering of a single mode LA phonon wave packet near the ends of the inner nanotube provides a net unbalanced force that, if large enough, initiates thermophoresis. By applying a coherent phonon pulse on the outer tube, which generalizes the single mode phonon wave packet, we are able to achieve thermophoresis in a carbon nanotube oscillator. We also find the nature of the unbalanced force on end-atoms to be qualitatively similar to that under an imposed thermal gradient. The thermodiffusion coefficient obtained for a range of thermal gradients and core lengths suggest that LA phonon scattering is the dominant mechanism for thermophoresis in longer cores, whereas for shorter cores, it is the highly diffusive mechanism that provides the effective force.

  18. Phonon stop bands in amorphous superlattices

    NASA Astrophysics Data System (ADS)

    Koblinger, O.; Mebert, J.; Dittrich, E.; Döttinger, S.; Eisenmenger, W.; Santos, P. V.; Ley, L.

    1987-06-01

    In periodically layered media the phonon-dispersion relation shows energy ranges in which phonon propagation is not possible. The existence of such phonon stop bands in crystalline superlattices has been observed in work by V. Narayanamurti, H. L. Störmer, M. A. Chin, A. C. Gossard, and W. Wiegman [Phys. Rev. Lett. 43, 2012 (1979)]. In this Communication we report the observation of phonon stop bands in amorphous superlattices. The filter characteristic of these amorphous superlattices is much sharper than in the case of the crystalline superlattices studied earlier. The investigated superlattices have been prepared by alternating evaporation of Si and SiO2 layers as well as by plasma-enhanced chemical vapor deposition of a-Si:H/a-SiNx:H films in a glow-discharge reactor.

  19. Probing Phonons in Plutonium

    NASA Astrophysics Data System (ADS)

    Wong, Joe

    2004-03-01

    The phonon spectra of plutonium and its alloys have been sought after in the past few decades following the discovery of this actinide element in 1941, but with no success. This was due to a combination of the high neutron absorption cross section of 239Pu, the common isotope, and non-availability of large single crystals of any Pu-bearing materials. We have recent designed a high resolution inelastic x-ray scattering experiment using a bright synchrotron x-ray beam at the European Sychrotron Radiation Facility (ESRF), Grenoble and mapped the full phonon dispersion curves of an fcc delta-phase polycrystalline Pu-Ga alloy (1). Several unusual features including, a large elastic anisotropy, a small shear elastic modulus C', a Kohn-like anomaly in the T1[011] branch, and a pronounced softening of the [111] transverse modes are found. These features can be related to the phase transitions of plutonium and to strong coupling between the lattice structure and the 5f valence instabilities. Our results also provide a critical test for theoretical treatments of highly correlated 5f electron systems as exemplified by recent dynamical mean field theory (DMFT) calculations for d-plutonium.(2) This work was performed in collaboration with Dr. M. Krisch (ESRF)) and Prof. T.-C. Chiang (UIU), and under the auspices of the U. S. Department of Energy by the University of California, Lawrence Livermore National Laboratory under Contract No. W-7405-Eng-48. 1. Joe Wong et al. Science, vol.301, 1078 (2003) 2. X. Dai et al. Science, vol.300, 953 (2003)

  20. Asymmetric propagation using enhanced self-demodulation in a chirped phononic crystal

    NASA Astrophysics Data System (ADS)

    Cebrecos, A.; Jiménez, N.; Romero-García, V.; Picó, R.; Sánchez-Morcillo, V. J.; García-Raffi, L. M.

    2016-12-01

    Asymmetric propagation of acoustic waves is theoretically reported in a chirped phononic crystal made of the combination of two different nonlinear solids. The dispersion of the system is spatially dependent and allows the rainbow trapping inside the structure. Nonlinearity is used to activate the self-demodulation effect, which is enhanced due to the particular dispersion characteristics of the system. The performed numerical study reveals an efficient generation of the demodulated wave, up to 15% in terms of the pressure amplitude, as well as strong attenuation for undesired frequency components above the cut-off frequency. The obtained energy rectification ratio is in the order of 104 for the whole range of amplitudes employed in this work, indicating the robustness of the asymmetry and non-reciprocity of the proposed device for a wide operational range.

  1. Probing phonons in plutonium

    SciTech Connect

    Wong, Joe; Krisch, M.; Farber, D.; Occelli, F.; Schwartz, A.; Chiang, T.C.; Wall, M.; Boro, C.; Xu, Ruqing

    2010-11-16

    Plutonium (Pu) is well known to have complex and unique physico-chemical properties. Notably, the pure metal exhibits six solid-state phase transformations with large volume expansions and contractions along the way to the liquid state: {alpha} {yields} {beta} {yields} {gamma} {yields} {delta} {yields} {delta}{prime} {yields} {var_epsilon} {yields} liquid. Unalloyed Pu melts at a relatively low temperature {approx}640 C to yield a higher density liquid than that of the solid from which it melts, (Figure 1). Detailed understanding of the properties of plutonium and plutonium-based alloys is critical for the safe handling, utilization, and long-term storage of these important, but highly toxic materials. However, both technical and and safety issues have made experimental observations extremely difficult. Phonon dispersion curves (PDCs) are key experimenta l data to the understanding of the basic properties of Pu materials such as: force constants, sound velocities, elastic constants, thermodynamics, phase stability, electron-phonon coupling, structural relaxation, etc. However, phonon dispersion curves (PDCs) in plutonium (Pu) and its alloys have defied measurement for the past few decades since the discovery of this element in 1941. This is due to a combination of the high thermal-neutron absorption cross section of plutonium and the inability to grow the large single crystals (with dimensions of a few millimeters) necessary for inelastic neutron scattering. Theoretical simulations of the Pu PDC continue to be hampered by the lack of suitable inter -atomic potentials. Thus, until recently the PDCs for Pu and its alloys have remained unknown experimentally and theoretically. The experimental limitations have recently been overcome by using a tightly focused undulator x-ray micro-beam scattered from single -grain domains in polycrystalline specimens. This experimental approach has been applied successfully to map the complete PDCs of an fcc d-Pu-Ga alloy using the

  2. Flexural-Phonon Scattering Induced by Electrostatic Gating in Graphene

    NASA Astrophysics Data System (ADS)

    Gunst, Tue; Kaasbjerg, Kristen; Brandbyge, Mads

    2017-01-01

    Graphene has an extremely high carrier mobility partly due to its planar mirror symmetry inhibiting scattering by the highly occupied acoustic flexural phonons. Electrostatic gating of a graphene device can break the planar mirror symmetry, yielding a coupling mechanism to the flexural phonons. We examine the effect of the gate-induced one-phonon scattering on the mobility for several gate geometries and dielectric environments using first-principles calculations based on density functional theory and the Boltzmann equation. We demonstrate that this scattering mechanism can be a mobility-limiting factor, and show how the carrier density and temperature scaling of the mobility depends on the electrostatic environment. Our findings may explain the high deformation potential for in-plane acoustic phonons extracted from experiments and, furthermore, suggest a direct relation between device symmetry and resulting mobility.

  3. Reduction of Thermal Conductivity by Nanoscale 3D Phononic Crystal

    PubMed Central

    Yang, Lina; Yang, Nuo; Li, Baowen

    2013-01-01

    We studied how the period length and the mass ratio affect the thermal conductivity of isotopic nanoscale three-dimensional (3D) phononic crystal of Si. Simulation results by equilibrium molecular dynamics show isotopic nanoscale 3D phononic crystals can significantly reduce the thermal conductivity of bulk Si at high temperature (1000 K), which leads to a larger ZT than unity. The thermal conductivity decreases as the period length and mass ratio increases. The phonon dispersion curves show an obvious decrease of group velocities in 3D phononic crystals. The phonon's localization and band gap is also clearly observed in spectra of normalized inverse participation ratio in nanoscale 3D phononic crystal. PMID:23378898

  4. Reduction of thermal conductivity by nanoscale 3D phononic crystal.

    PubMed

    Yang, Lina; Yang, Nuo; Li, Baowen

    2013-01-01

    We studied how the period length and the mass ratio affect the thermal conductivity of isotopic nanoscale three-dimensional (3D) phononic crystal of Si. Simulation results by equilibrium molecular dynamics show isotopic nanoscale 3D phononic crystals can significantly reduce the thermal conductivity of bulk Si at high temperature (1000 K), which leads to a larger ZT than unity. The thermal conductivity decreases as the period length and mass ratio increases. The phonon dispersion curves show an obvious decrease of group velocities in 3D phononic crystals. The phonon's localization and band gap is also clearly observed in spectra of normalized inverse participation ratio in nanoscale 3D phononic crystal.

  5. Hot carrier and hot phonon coupling during ultrafast relaxation of photoexcited electrons in graphene

    SciTech Connect

    Iglesias, J. M.; Martín, M. J.; Pascual, E.; Rengel, R.

    2016-01-25

    We study, by means of a Monte Carlo simulator, the hot phonon effect on the relaxation dynamics in photoexcited graphene and its quantitative impact as compared with considering an equilibrium phonon distribution. Our multi-particle approach indicates that neglecting the hot phonon effect significantly underestimates the relaxation times in photoexcited graphene. The hot phonon effect is more important for a higher energy of the excitation pulse and photocarrier densities between 1 and 3 × 10{sup 12 }cm{sup −2}. Acoustic intervalley phonons play a non-negligible role, and emitted phonons with wavelengths limited up by a maximum (determined by the carrier concentration) induce a slower carrier cooling rate. Intrinsic phonon heating is damped in graphene on a substrate due to the additional cooling pathways, with the hot phonon effect showing a strong inverse dependence with the carrier density.

  6. Optic phonons and anisotropic thermal conductivity in hexagonal Ge2Sb2Te5

    SciTech Connect

    Mukhopadhyay, Saikat; Lindsay, Lucas R.; Singh, David

    2016-11-16

    The lattice thermal conductivity ($κ$) of hexagonal Ge2Sb2Tesub>5 (h-GST) is studied via direct first-principles calculations. We find significant intrinsic anisotropy of ( $κ$a/$κ$c~2) of $κ$ in bulk h-GST along different transport directions. The dominant contribution to$κ$ is from optic phonons, ~75%. This is extremely unusual as the acoustic phonon modes carry most of the heat in typical semiconductors and insulators with small unit cells. Very recently, Lee et. al. observed anisotropic in GST thin films and attributed this to thermal resistance of amorphous regions near grain boundaries. However, our results suggest an additional strong intrinsic anisotropy for the pure hexagonal phase. This derives from bonding anisotropy along different crystal directions, specifically from weak interlayer coupling, which gives anisotropic phonon dispersions. The phonon spectrum of h-GST has very dispersive optic branches with higher group velocities along the a-axis as compared to flat optic bands along the c-axis. The importance of optic mode contributions for the thermal conductivity in low-$κ$ h-GST is unusual, and development of fundamental physical understanding of these contributions may be critical to better understanding of thermal conduction in other complex layered materials.

  7. Rainbow trapping of ultrasonic guided waves in chirped phononic crystal plates.

    PubMed

    Tian, Zhenhua; Yu, Lingyu

    2017-01-05

    The rainbow trapping effect has been demonstrated in electromagnetic and acoustic waves. In this study, rainbow trapping of ultrasonic guided waves is achieved in chirped phononic crystal plates that spatially modulate the dispersion, group velocity, and stopband. The rainbow trapping is related to the progressively slowing group velocity, and the extremely low group velocity near the lower boundary of a stopband that gradually varies in chirped phononic crystal plates. As guided waves propagate along the phononic crystal plate, waves gradually slow down and finally stop forward propagating. The energy of guided waves is concentrated at the low velocity region near the stopband. Moreover, the guided wave energy of different frequencies is concentrated at different locations, which manifests as rainbow guided waves. We believe implementing the rainbow trapping will open new paradigms for guiding and focusing of guided waves. Moreover, the rainbow guided waves with energy concentration and spatial separation of frequencies may have potential applications in nondestructive evaluation, spatial wave filtering, energy harvesting, and acoustofluidics.

  8. Rainbow trapping of ultrasonic guided waves in chirped phononic crystal plates

    NASA Astrophysics Data System (ADS)

    Tian, Zhenhua; Yu, Lingyu

    2017-01-01

    The rainbow trapping effect has been demonstrated in electromagnetic and acoustic waves. In this study, rainbow trapping of ultrasonic guided waves is achieved in chirped phononic crystal plates that spatially modulate the dispersion, group velocity, and stopband. The rainbow trapping is related to the progressively slowing group velocity, and the extremely low group velocity near the lower boundary of a stopband that gradually varies in chirped phononic crystal plates. As guided waves propagate along the phononic crystal plate, waves gradually slow down and finally stop forward propagating. The energy of guided waves is concentrated at the low velocity region near the stopband. Moreover, the guided wave energy of different frequencies is concentrated at different locations, which manifests as rainbow guided waves. We believe implementing the rainbow trapping will open new paradigms for guiding and focusing of guided waves. Moreover, the rainbow guided waves with energy concentration and spatial separation of frequencies may have potential applications in nondestructive evaluation, spatial wave filtering, energy harvesting, and acoustofluidics.

  9. Rainbow trapping of ultrasonic guided waves in chirped phononic crystal plates

    PubMed Central

    Tian, Zhenhua; Yu, Lingyu

    2017-01-01

    The rainbow trapping effect has been demonstrated in electromagnetic and acoustic waves. In this study, rainbow trapping of ultrasonic guided waves is achieved in chirped phononic crystal plates that spatially modulate the dispersion, group velocity, and stopband. The rainbow trapping is related to the progressively slowing group velocity, and the extremely low group velocity near the lower boundary of a stopband that gradually varies in chirped phononic crystal plates. As guided waves propagate along the phononic crystal plate, waves gradually slow down and finally stop forward propagating. The energy of guided waves is concentrated at the low velocity region near the stopband. Moreover, the guided wave energy of different frequencies is concentrated at different locations, which manifests as rainbow guided waves. We believe implementing the rainbow trapping will open new paradigms for guiding and focusing of guided waves. Moreover, the rainbow guided waves with energy concentration and spatial separation of frequencies may have potential applications in nondestructive evaluation, spatial wave filtering, energy harvesting, and acoustofluidics. PMID:28054601

  10. Rainbow trapping of ultrasonic guided waves in chirped phononic crystal plates

    DOE PAGES

    Tian, Zhenhua; Yu, Lingyu

    2017-01-05

    The rainbow trapping effect has been demonstrated in electromagnetic and acoustic waves. In this study, rainbow trapping of ultrasonic guided waves is achieved in chirped phononic crystal plates that spatially modulate the dispersion, group velocity, and stopband. The rainbow trapping is related to the progressively slowing group velocity, and the extremely low group velocity near the lower boundary of a stopband that gradually varies in chirped phononic crystal plates. As guided waves propagate along the phononic crystal plate, waves gradually slow down and finally stop forward propagating. The energy of guided waves is concentrated at the low velocity region nearmore » the stopband. Moreover, the guided wave energy of different frequencies is concentrated at different locations, which manifests as rainbow guided waves. We believe implementing the rainbow trapping will open new paradigms for guiding and focusing of guided waves. Furthermore, the rainbow guided waves with energy concentration and spatial separation of frequencies may have potential applications in nondestructive evaluation, spatial wave filtering, energy harvesting, and acoustofluidics.« less

  11. Phononic Frequency Comb via Intrinsic Three-Wave Mixing.

    PubMed

    Ganesan, Adarsh; Do, Cuong; Seshia, Ashwin

    2017-01-20

    Optical frequency combs have resulted in significant advances in optical frequency metrology and found wide applications in precise physical measurements and molecular fingerprinting. A direct analogue of frequency combs in the phononic or acoustic domain has not been reported to date. In this Letter, we report the first clear experimental evidence for a phononic frequency comb. We show that the phononic frequency comb is generated through the intrinsic coupling of a driven phonon mode with an autoparametrically excited subharmonic mode. The experiments depict the comb generation process evidenced by a spectral response consisting of equally spaced discrete and phase coherent comb lines. Through systematic experiments at different drive frequencies and amplitudes, we portray the well-connected process of phononic frequency comb formation and define the attributes to control the features associated with comb formation in such a system. In addition to the demonstration of frequency comb, the interplay between the nonlinear resonances and the well-known Duffing phenomenon is also observed.

  12. Phononic Frequency Comb via Intrinsic Three-Wave Mixing

    NASA Astrophysics Data System (ADS)

    Ganesan, Adarsh; Do, Cuong; Seshia, Ashwin

    2017-01-01

    Optical frequency combs have resulted in significant advances in optical frequency metrology and found wide applications in precise physical measurements and molecular fingerprinting. A direct analogue of frequency combs in the phononic or acoustic domain has not been reported to date. In this Letter, we report the first clear experimental evidence for a phononic frequency comb. We show that the phononic frequency comb is generated through the intrinsic coupling of a driven phonon mode with an autoparametrically excited subharmonic mode. The experiments depict the comb generation process evidenced by a spectral response consisting of equally spaced discrete and phase coherent comb lines. Through systematic experiments at different drive frequencies and amplitudes, we portray the well-connected process of phononic frequency comb formation and define the attributes to control the features associated with comb formation in such a system. In addition to the demonstration of frequency comb, the interplay between the nonlinear resonances and the well-known Duffing phenomenon is also observed.

  13. Landau-Zener-Stückelberg Interferometry in Quantum Dots with Fast Rise Times: Evidence for Coherent Phonon Driving

    NASA Astrophysics Data System (ADS)

    Korkusinski, M.; Studenikin, S. A.; Aers, G.; Granger, G.; Kam, A.; Sachrajda, A. S.

    2017-02-01

    Manipulating qubits via electrical pulses in a piezoelectric material such as GaAs can be expected to generate incidental acoustic phonons. In this Letter we determine theoretically and experimentally the consequences of these phonons for semiconductor spin qubits using Landau-Zener-Stückelberg interferometry. Theoretical calculations predict that phonons in the presence of the spin-orbit interaction produce both phonon-Rabi fringes and accelerated evolution at the singlet-triplet anticrossing. Observed features confirm the influence of these mechanisms. Additionally, evidence is found that the pulsed gates themselves act as phonon cavities increasing the influence of phonons under specific resonant conditions.

  14. Landau-Zener-Stückelberg Interferometry in Quantum Dots with Fast Rise Times: Evidence for Coherent Phonon Driving.

    PubMed

    Korkusinski, M; Studenikin, S A; Aers, G; Granger, G; Kam, A; Sachrajda, A S

    2017-02-10

    Manipulating qubits via electrical pulses in a piezoelectric material such as GaAs can be expected to generate incidental acoustic phonons. In this Letter we determine theoretically and experimentally the consequences of these phonons for semiconductor spin qubits using Landau-Zener-Stückelberg interferometry. Theoretical calculations predict that phonons in the presence of the spin-orbit interaction produce both phonon-Rabi fringes and accelerated evolution at the singlet-triplet anticrossing. Observed features confirm the influence of these mechanisms. Additionally, evidence is found that the pulsed gates themselves act as phonon cavities increasing the influence of phonons under specific resonant conditions.

  15. Acoustoelectric effect in graphene with degenerate energy dispersion

    NASA Astrophysics Data System (ADS)

    Dompreh, K. A.; Mensah, N. G.; Mensah, S. Y.

    2017-01-01

    Acoustoelectric current (jac) in Free-Standing Graphene (FSG) having degenerate energy dispersion at low temperatures T ≪TBG (TBG is the Block-Gruneisen temperature) was studied theoretically. We considered electron interaction with in-plain acoustic phonons in the hypersound regime (sound vibration in the range 109 -1012 Hz). The obtained expression for jac was numerically analyzed for various temperatures (T) and frequencies (ωq) and graphically presented. The non-linear dependence of jac on ωq varied with temperature. This qualitatively agreed with an experimentally obtained result which deals with temperature dependent acoustoelectric current in graphene [21].

  16. Band structures in a two-dimensional phononic crystal with rotational multiple scatterers

    NASA Astrophysics Data System (ADS)

    Song, Ailing; Wang, Xiaopeng; Chen, Tianning; Wan, Lele

    2017-03-01

    In this paper, the acoustic wave propagation in a two-dimensional phononic crystal composed of rotational multiple scatterers is investigated. The dispersion relationships, the transmission spectra and the acoustic modes are calculated by using finite element method. In contrast to the system composed of square tubes, there exist a low-frequency resonant bandgap and two wide Bragg bandgaps in the proposed structure, and the transmission spectra coincide with band structures. Specially, the first bandgap is based on locally resonant mechanism, and the simulation results agree well with the results of electrical circuit analogy. Additionally, increasing the rotation angle can remarkably influence the band structures due to the transfer of sound pressure between the internal and external cavities in low-order modes, and the redistribution of sound pressure in high-order modes. Wider bandgaps are obtained in arrays composed of finite unit cells with different rotation angles. The analysis results provide a good reference for tuning and obtaining wide bandgaps, and hence exploring the potential applications of the proposed phononic crystal in low-frequency noise insulation.

  17. Optical studies of terahertz phonons dynamics in small-grain polycrystalline corundum

    NASA Astrophysics Data System (ADS)

    Feofilov, S. P.; Kaplyanskii, A. A.; Kulinkin, A. B.; Zakharchenya, R. I.

    1999-03-01

    The dynamics of terahertz acoustic phonons generated by optical pumping in ceramic-like α-Al 2O 3 with grain size ∼100 nm produced with the help of sol-gel technology was studied with the technique of optical detection of phonons by observation of probe Cr 3+ and Mn 4+ ions fluorescence. The dynamics of phonon distribution is very slow (∼ms) and drastically differs from that in regular α-Al 2O 3 ceramics with micron grain size and is similar to that observed earlier in oxide glasses. The results are discussed in the framework of studies of phonons in different structured and spatially restricted Al 2O 3 materials with different ratios between phonon wavelength λ and crystallite size a. It is shown that the acoustic mismatch model which describes phonon scattering in regular ceramics is not valid for small-grain sol-gel produced ceramics-like material.

  18. Broadband magnetoelastic coupling in magnonic-phononic crystals for high-frequency nanoscale spin-wave generation

    NASA Astrophysics Data System (ADS)

    Graczyk, Piotr; Kłos, Jarosław; Krawczyk, Maciej

    2017-03-01

    Spin waves are promising candidates for information carriers in advanced technology. The interactions between spin waves and acoustic waves in magnetic nanostructures are of much interest because of their potential application for spin-wave generation, amplification, and transduction. We investigate numerically the dynamics of magnetoelastic excitations in a one-dimensional magnonic-phononic crystal consisting of alternating layers of permalloy and cobalt. We use the plane-wave method and the finite-element method for frequency- and time-domain simulations, respectively. The studied structure is optimized for hybridization of specific spin-wave and acoustic dispersion branches in the entire Brillouin zone in a broad frequency range. We show that this type of periodic structure can be used for efficient generation of high-frequency spin waves.

  19. Phonon engineering for nanostructures.

    SciTech Connect

    Aubry, Sylvie; Friedmann, Thomas Aquinas; Sullivan, John Patrick; Peebles, Diane Elaine; Hurley, David H.; Shinde, Subhash L.; Piekos, Edward Stanley; Emerson, John Allen

    2010-01-01

    Understanding the physics of phonon transport at small length scales is increasingly important for basic research in nanoelectronics, optoelectronics, nanomechanics, and thermoelectrics. We conducted several studies to develop an understanding of phonon behavior in very small structures. This report describes the modeling, experimental, and fabrication activities used to explore phonon transport across and along material interfaces and through nanopatterned structures. Toward the understanding of phonon transport across interfaces, we computed the Kapitza conductance for {Sigma}29(001) and {Sigma}3(111) interfaces in silicon, fabricated the interfaces in single-crystal silicon substrates, and used picosecond laser pulses to image the thermal waves crossing the interfaces. Toward the understanding of phonon transport along interfaces, we designed and fabricated a unique differential test structure that can measure the proportion of specular to diffuse thermal phonon scattering from silicon surfaces. Phonon-scale simulation of the test ligaments, as well as continuum scale modeling of the complete experiment, confirmed its sensitivity to surface scattering. To further our understanding of phonon transport through nanostructures, we fabricated microscale-patterned structures in diamond thin films.

  20. Coherent optical phonon oscillation and possible electronic softening in WTe2 crystals.

    PubMed

    He, Bin; Zhang, Chunfeng; Zhu, Weida; Li, Yufeng; Liu, Shenghua; Zhu, Xiyu; Wu, Xuewei; Wang, Xiaoyong; Wen, Hai-Hu; Xiao, Min

    2016-07-26

    A rapidly-growing interest in WTe2 has been triggered by the giant magnetoresistance effect discovered in this unique system. While many efforts have been made towards uncovering the electron- and spin-relevant mechanisms, the role of lattice vibration remains poorly understood. Here, we study the coherent vibrational dynamics in WTe2 crystals by using ultrafast pump-probe spectroscopy. The oscillation signal in time domain in WTe2 has been ascribed as due to the coherent dynamics of the lowest energy A1 optical phonons with polarization- and wavelength-dependent measurements. With increasing temperature, the phonon energy decreases due to anharmonic decay of the optical phonons into acoustic phonons. Moreover, a significant drop (15%) of the phonon energy with increasing pump power is observed which is possibly caused by the lattice anharmonicity induced by electronic excitation and phonon-phonon interaction.

  1. Coherent optical phonon oscillation and possible electronic softening in WTe2 crystals

    PubMed Central

    He, Bin; Zhang, Chunfeng; Zhu, Weida; Li, Yufeng; Liu, Shenghua; Zhu, Xiyu; Wu, Xuewei; Wang, Xiaoyong; Wen, Hai-hu; Xiao, Min

    2016-01-01

    A rapidly-growing interest in WTe2 has been triggered by the giant magnetoresistance effect discovered in this unique system. While many efforts have been made towards uncovering the electron- and spin-relevant mechanisms, the role of lattice vibration remains poorly understood. Here, we study the coherent vibrational dynamics in WTe2 crystals by using ultrafast pump-probe spectroscopy. The oscillation signal in time domain in WTe2 has been ascribed as due to the coherent dynamics of the lowest energy A1 optical phonons with polarization- and wavelength-dependent measurements. With increasing temperature, the phonon energy decreases due to anharmonic decay of the optical phonons into acoustic phonons. Moreover, a significant drop (15%) of the phonon energy with increasing pump power is observed which is possibly caused by the lattice anharmonicity induced by electronic excitation and phonon-phonon interaction. PMID:27457385

  2. Ultrafast optical generation of coherent phonons in CdTe1-xSex quantum dots

    NASA Astrophysics Data System (ADS)

    Bragas, A. V.; Aku-Leh, C.; Costantino, S.; Ingale, Alka; Zhao, J.; Merlin, R.

    2004-05-01

    We report on the impulsive generation of coherent optical phonons in CdTe0.68Se0.32 nanocrystallites embedded in a glass matrix. Pump-probe experiments using femtosecond laser pulses were performed by tuning the laser central energy to resonate with the absorption edge of the nanocrystals. We identify two longitudinal optical phonons, one longitudinal acoustic phonon and a fourth mode of a mixed longitudinal-transverse nature. The amplitude of the optical phonons as a function of the laser central energy exhibits a resonance that is well described by a model based on impulsive stimulated Raman scattering. The phases of the coherent phonons reveal coupling between different modes. At low power density excitations, the frequency of the optical coherent phonons deviates from values obtained from spontaneous Raman scattering. This behavior is ascribed to the presence of electronic impurity states which modify the nanocrystal dielectric function and, thereby, the frequency of the infrared-active phonons.

  3. Strong acoustic coupling to a superconducting qubit

    NASA Astrophysics Data System (ADS)

    Gustafsson, Martin; Aref, Thomas; Frisk Kockum, Anton; Ekström, Maria; Johansson, Göran; Delsing, Per

    2014-03-01

    Micromechanical resonators can be used to store quantum information, as shown in several recent experiments. These resonators typically have the form of membranes or beams, and phonons are localized to their vibrational eigenmodes. We present a different kind of mechanical quantum device, where propagating phonons serve as carriers for quantum information. At the core of our device is a superconducting qubit, designed to couple to Surface Acoustic Waves (SAW) in the underlying substrate through the piezoelectric effect. This type of coupling can be very strong, and in our case exceeds the coupling to any external electromagnetic modes. The acoustic waves propagate freely on the surface of the substrate, and we use a remote electro-acoustic transducer to address the qubit acoustically and listen to its emission of phonons. This presentation focuses on the basic properties of our acoustic quantum system, and we include experimental data that demonstrate the quantized coupling between the qubit and the propagating acoustic waves.

  4. Phonons in NaO/sub 2/ near the order-disorder transition

    SciTech Connect

    Wakabayashi, N.; Alefeld, B.; Buhrer, W.; Smith, H.G.

    1982-10-15

    The acoustic phonons in cubic NaO/sub 2/ have been studied above and below the order-disorder transition by inelastic neutron scattering. Above the transition the O/sub 2/ /sup -/ ions are disordered and undergoing rapid reorientation about the body diagonals. This reorientation couples with and affects certain acoustic modes in the crystal. The results are described in terms of a phonon-pseudospin coupling theory.

  5. Research on micro-sized acoustic bandgap structures.

    SciTech Connect

    Fleming, James Grant; McCormick, Frederick Bossert; Su, Mehmet F.; El-Kady, Ihab Fathy; Olsson, Roy H., III; Tuck, Melanie R.

    2010-01-01

    Phononic crystals (or acoustic crystals) are the acoustic wave analogue of photonic crystals. Here a periodic array of scattering inclusions located in a homogeneous host material forbids certain ranges of acoustic frequencies from existence within the crystal, thus creating what are known as acoustic (or phononic) bandgaps. The vast majority of phononic crystal devices reported prior to this LDRD were constructed by hand assembling scattering inclusions in a lossy viscoelastic medium, predominantly air, water or epoxy, resulting in large structures limited to frequencies below 1 MHz. Under this LDRD, phononic crystals and devices were scaled to very (VHF: 30-300 MHz) and ultra (UHF: 300-3000 MHz) high frequencies utilizing finite difference time domain (FDTD) modeling, microfabrication and micromachining technologies. This LDRD developed key breakthroughs in the areas of micro-phononic crystals including physical origins of phononic crystals, advanced FDTD modeling and design techniques, material considerations, microfabrication processes, characterization methods and device structures. Micro-phononic crystal devices realized in low-loss solid materials were emphasized in this work due to their potential applications in radio frequency communications and acoustic imaging for medical ultrasound and nondestructive testing. The results of the advanced modeling, fabrication and integrated transducer designs were that this LDRD produced the 1st measured phononic crystals and phononic crystal devices (waveguides) operating in the VHF (67 MHz) and UHF (937 MHz) frequency bands and established Sandia as a world leader in the area of micro-phononic crystals.

  6. Thermal transport in phononic crystals: The role of zone folding effect

    NASA Astrophysics Data System (ADS)

    Dechaumphai, Edward; Chen, Renkun

    2012-04-01

    Recent experiments [Yu et al., Nature Nanotech 5, 718 (2010); Tang et al., Nano Lett. 10, 4279 (2010); Hopkins etal., Nano Lett. 11, 107(2011)] on silicon based nanoscale phononic crystals demonstrated substantially reduced thermal conductivity compared to bulk Si, which cannot be explained by incoherent phonon boundary scattering within the Boltzmann Transport Equation (BTE). In this paper, partial coherent treatment of phonons, where phonons are regarded as either wave or particles depending on their frequencies, was considered. Phonons with mean free path smaller than the characteristic size of phononic crystals are treated as particles and the transport in this regime is modeled by BTE with phonon boundary scattering taken into account. On the other hand, phonons with mean free path longer than the characteristic size are treated as waves. In this regime, phonon dispersion relations are computed using the Finite Difference Time Domain (FDTD) method and are found to be modified due to the zone folding effect. The new phonon spectra are then used to compute phonon group velocity and density of states for thermal conductivity modeling. Our partial coherent model agrees well with the recent experimental results on in-plane thermal conductivity of phononic crystals. Our study highlights the importance of zone folding effect on thermal transport in phononic crystals.

  7. Study of the thermodynamic properties of CeO{sub 2} from ab initio calculations: The effect of phonon-phonon interaction

    SciTech Connect

    Niu, Zhen-Wei; Zeng, Zhao-Yi; Hu, Cui-E; Cai, Ling-Cang; Chen, Xiang-Rong

    2015-01-07

    The thermodynamic properties of CeO{sub 2} have been reevaluated by a simple but accurate scheme. All our calculations are based on the self-consistent ab initio lattice dynamical (SCAILD) method that goes beyond the quasiharmonic approximation. Through this method, the effects of phonon-phonon interactions are included. The obtained thermodynamic properties and phonon dispersion relations are in good agreement with experimental data when considering the correction of phonon-phonon interaction. We find that the correction of phonon-phonon interaction is equally important and should not be neglected. At last, by comparing with quasiharmonic approximation, the present scheme based on SCAILD method is probably more suitable for high temperature systems.

  8. Design and Optimization of Phononic Crystals and Metamaterials for Flow Control and Other Applications

    NASA Astrophysics Data System (ADS)

    Bilal, Osama R.

    Transmission of everyday sound and heat can be traced back to a physical particle, or wave, called a "phonon". Understanding, analyzing and manipulating phonons across multiple scales/disciplines can be achieved using phononic materials. That is a class of material systems featuring a basic pattern that repeats spatially. Among many qualities, it exhibits distinct frequency characteristics such as band gaps, where vibrational waves of certain frequencies are prohibited from propagation. These properties can benefit a multitude of applications, ranging from vibration isolation and converting waste heat into electricity to exotic concepts like acoustic cloaking. Using unit-cell design and optimization, phononic materials/devices with extraordinary properties may be realized. Since many of these applications are based on band-gap utilization, a critical design objective is to widen band-gap size or precisely synthesize its characteristics. Approaching this problem at the unit cell level is advantageous in many aspects, mostly because it provides a complete picture of the intrinsic local dynamics which is often obscured when analyzing the structure as a whole. Moreover, it is computationally less expensive than designing an entire structure. Unit-cell dispersion engineering is also scale independent; an optimized unit cell may be used to manipulate waves ranging from a few Hz to GHz, or higher, with proper scaling. In order to keep the structure/device size as small as possible, the band-gap central frequency is tuned to be as low as possible. The objective of this thesis is to explore and advance unit-cell design and optimization of phononic materials in one, two and three-dimensions for a broad range of applications. In particular, an application for flow control is investigated where a phononic material is shown to manipulate and alter a flow field in a favorable manner. Results involving unit-cell design and coupled fluid-structure simulations (as part of a

  9. Shear Bloch waves and coupled phonon-polariton in periodic piezoelectric waveguides.

    PubMed

    Piliposyan, D G; Ghazaryan, K B; Piliposian, G T

    2014-02-01

    Coupled electro-elastic SH waves propagating in a periodic piezoelectric finite-width waveguide are considered in the framework of the full system of Maxwell's electrodynamic equations. We investigate Bloch-Floquet waves under homogeneous or alternating boundary conditions for the elastic and electromagnetic fields along the guide walls. Zero frequency stop bands, trapped modes as well as some anomalous features due to piezoelectricity are identified. For mixed boundary conditions, by modulating the ratio of the length of the unit cell to the width of the waveguide, the minimum widths of the stop bands can be moved to the middle of the Brillouin zone. The dispersion equation has been investigated also for phonon-polariton band gaps. It is shown that for waveguides at acoustic frequencies, acousto-optic coupling gives rise to polariton behavior at wavelengths much larger than the length of the unit cell but at optical frequencies polariton resonance occurs at wavelengths comparable with the period of the waveguide.

  10. Structure of crystalline oxide ceramics studied by phonon spectroscopy

    SciTech Connect

    Kaminskii, Alexandr A; Taranov, A V; Khazanov, E N

    2013-03-31

    This paper describes a method for gaining detailed insight into the structure and phonon spectrum of polycrystalline oxide ceramics. We examine how the diffusion coefficient of subterahertz phonons is related to the properties of a system of grain boundaries and to the grain size and structure and demonstrate that the temperature dependence of the phonon diffusion coefficient at liquid-helium temperatures is determined by the spectral properties of the intergranular layer, which allows one to estimate the volumeaveraged intergranular layer thickness and acoustic impedance. We also analyse the effect of plastic deformation via twinning on the formation of the structure of grains and intergranular layers, which determine the thermophysical, acoustic and optical properties of ceramic materials. (extreme light fields and their applications)

  11. Molecular Detection and Phonon Filtering in Heat-Transfer Spectroscopy

    NASA Astrophysics Data System (ADS)

    Walczak, Kamil; Yerkes, Kirk

    2014-03-01

    We examine heat transport carried by acoustic phonons in the systems composed of nanoscale chains of masses coupled to two thermal baths of different temperatures. Thermal conductance is obtained by using linearized Landauer formula for heat flux with phonon transmission probability calculated within atomistic Green's functions (AGF) method. AGF formalism is extended onto dissipative chains of masses with harmonic coupling beyond nearest-neighbor approximation, while atomistic description of heat reservoirs is also included into computational scheme. The resonant structure of phonon transmission spectrum is analyzed with respect to reservoir-dimensionality effects, molecular damping, and mass-to-mass harmonic coupling. Analysis of transmission zeros (antiresonances) and their accompanied Fano-shape resonances are discussed as a result of interference effects between different vibrational modes. Specifically, we show that the heat-transfer-based characterization method may be used to identify individual molecules or filter out specific phonon modes from the whole frequency spectrum. This work is supported by AFOSR grant.

  12. The anharmonic phonon decay rate in group-III nitrides

    NASA Astrophysics Data System (ADS)

    Srivastava, G. P.

    2009-04-01

    Measured lifetimes of hot phonons in group-III nitrides have been explained theoretically by considering three-phonon anharmonic interaction processes. The basic ingredients of the theory include full phonon dispersion relations obtained from the application of an adiabatic bond charge model and crystal anharmonic potential within the isotropic elastic continuum model. The role of various decay routes, such as Klemens, Ridley, Vallée-Bogani and Barman-Srivastava channels, in determining the lifetimes of the Raman active zone-centre longitudinal optical (LO) modes in BN (zincblende structure) and A1(LO) modes in AlN, GaN and InN (wurtzite structure) has been quantified.

  13. First-Principles Calculation of forces and phonons in solid

    NASA Astrophysics Data System (ADS)

    Ning, Zhenhua; Shelton, William

    We have developed a multiple scattering theory approach to calculate Hellmann-Feynman forces and phonons via the calculation of the force constant and dynamical matrix. To demonstrate the accuracy and validity of our approach we compare with the ELK code, which is a full potential Linear Augmented Plane Wave (FLAPW) based method. As we will show our forces and phonon dispersion curves are in good agreement with the FLAPW code. This work lays the foundation for developing a first principles approach for calculation of phonons in substitutionally disordered materials.

  14. Temperature dependence of phonon-defect interactions: phonon scattering vs. phonon trapping

    PubMed Central

    Bebek, M. B.; Stanley, C. M.; Gibbons, T. M.; Estreicher, S. K.

    2016-01-01

    The interactions between thermal phonons and defects are conventionally described as scattering processes, an idea proposed almost a century ago. In this contribution, ab-initio molecular-dynamics simulations provide atomic-level insight into the nature of these interactions. The defect is the Si|X interface in a nanowire containing a δ-layer (X is C or Ge). The phonon-defect interactions are temperature dependent and involve the trapping of phonons for meaningful lengths of time in defect-related, localized, vibrational modes. No phonon scattering occurs and the momentum of the phonons released by the defect is unrelated to the momentum of the phonons that generated the excitation. The results are extended to the interactions involving only bulk phonons and to phonon-defect interactions at high temperatures. These do resemble scattering since phonon trapping occurs for a length of time short enough for the momentum of the incoming phonon to be conserved. PMID:27535463

  15. Phonon Analysis in Multiphonon Transitions

    NASA Astrophysics Data System (ADS)

    Huang, Kun; Gu, Zongquan

    In the investigation of multiphonon transitions, single-mode or single-frequency models are widely used. In view of the fact that such oversimplified models can be seriously inadequate, the present work bridges the gap between the complexity of the general formal theory and the simplicity required for concrete applications by introducing the concept of multi-frequency models. That is, the theory is so formulated that a general system can be approximated by multi-frequency models of any degree of elaboration. A statistical thermodynamic formalism is developed for treating such multi-frequency models, which, on the one hand, greatly reduces the labour of calculation with such models and, on the other hand, leads directly to a simple statistical distribution law for numbers of phonons of each frequency participating in a multiphonon transition. Applications of the theory to concrete models lead to certain general conclusions on frequency dispersion effects in multiphonon transitions. The use of the theory is further demonstrated by fully accounting for the paradoxical experimental results reported by Jia and Yen that the isotopic substitution of H by D in CsMn Cl3· 2H2O reduces the multiphonon nonradiative transition probability of excited Mn2+ ion by more than ten-fold, and yet leaves the corresponding luminescence phonon sideband little changed. In the last section of the paper, the relation between the statistical thermodynamic formalism and existing multiphonon transition theory is elucidated, thereby the theoretical basis of the statistical formalism becomes clearly defined.

  16. Effect of phonon focusing on Knudsen flow of phonon gas in single-crystal nanowires made of spintronics materials

    NASA Astrophysics Data System (ADS)

    Kuleev, I. I.; Bakharev, S. M.; Kuleev, I. G.; Ustinov, V. V.

    2017-01-01

    Effect of anisotropy of elastic energy on the phonon propagation in single-crystal nanowires made of Fe, Cu, MgO, InSb, and GaAs materials that are used to fabricate spintronics devices in the regime of the Knudsen flow of phonon gas has been studied. A new method of analyzing the focusing of quasi-transverse modes has been suggested, which made it possible to determine the average values of the densities of phonon states in the regions of focusing and defocusing slow and fast quasi-transverse modes. The effect of phonon focusing on the anisotropy of heat conductivity and lengths of the phonon free paths has been analyzed for all acoustic modes that exist in spintronics nanostructures. It has been shown that for all the nanowires investigated the angular dependences of the free paths of fast and slow transverse modes in the {100} and {110} planes correlate with the angular dependences of the densities of phonon states for these modes. Directions of the heat flux that ensure the maximum and minimum phonon heat conductivity in the nanowires have been determined.

  17. Optic phonon bandwidth and lattice thermal conductivity: The case of Li2X ( X=O , S, Se, Te)

    DOE PAGES

    Mukhopadhyay, S.; Lindsay, L.; Parker, D. S.

    2016-06-07

    Here, we examine the lattice thermal conductivities ( l) of Li2X (X=O, S, Se, Te) using a first-principles Peierls-Boltzmann transport methodology. We find low l values ranging between 12 and 30 W/m-K despite light Li atoms, a large mass difference between constituent atoms and tightly bunched acoustic branches, all features that give high l in other materials including BeSe (630 W/m-1K-1), BeTe (370 W/m-1K-1) and cubic BAs (3150 W/m-1K-1). Together these results suggest a missing ingredient in the basic guidelines commonly used to understand and predict l. Unlike typical simple systems (e.g., Si, GaAs, SiC), the dominant resistance to heat-carryingmore » acoustic phonons in Li2Se and Li2Te comes from interactions of these modes with two optic phonons. These interactions require significant bandwidth and dispersion of the optic branches, both present in Li2X materials. Finally, these considerations are important for the discovery and design of new materials for thermal management applications, and give a more comprehensive understanding of thermal transport in crystalline solids.« less

  18. Excitation of surface waves on one-dimensional solid–fluid phononic crystals and the beam displacement effect

    SciTech Connect

    Moiseyenko, Rayisa P.; Liu, Jingfei; Declercq, Nico F.; Benchabane, Sarah; Laude, Vincent

    2014-12-15

    The possibility of surface wave generation by diffraction of pressure waves on deeply corrugated one-dimensional phononic crystal gratings is studied both theoretically and experimentally. Generation of leaky surface waves, indeed, is generally invoked in the explanation of the beam displacement effect that can be observed upon reflection on a shallow grating of an acoustic beam of finite width. True surface waves of the grating, however, have a dispersion that lies below the sound cone in water. They thus cannot satisfy the phase-matching condition for diffraction from plane waves of infinite extent incident from water. Diffraction measurements indicate that deeply corrugated one-dimensional phononic crystal gratings defined in a silicon wafer are very efficient diffraction gratings. They also confirm that all propagating waves detected in water follow the grating law. Numerical simulations however reveal that in the sub-diffraction regime, acoustic energy of a beam of finite extent can be transferred to elastic waves guided at the surface of the grating. Their leakage to the specular direction along the grating surface explains the apparent beam displacement effect.

  19. Optical Generation and Detection of Local Nonequilibrium Phonons in Suspended Graphene

    NASA Astrophysics Data System (ADS)

    Sullivan, Sean; Vallabhaneni, Ajit; Kholmanov, Iskandar; Ruan, Xiulin; Murthy, Jayathi; Shi, Li

    2017-03-01

    The measured frequencies and intensities of different first- and second- order Raman peaks of suspended graphene are used to show that optical phonons and different acoustic phonon polarizations are driven out of local equilibrium inside a sub-micron laser spot. The experimental results are correlated with a first principles-based multiple temperature model to suggest a considerably lower equivalent local temperature of the flexural phonons than those of other phonon polarizations. The finding reveals weak coupling between the flexural modes with hot electrons and optical phonons. Since the ultrahigh intrinsic thermal conductivity of graphene has been largely attributed to contributions from the flexural phonons, the observed local non-equilibrium phenomena have important implications for understanding energy dissipation processes in graphene-based electronic and optoelectronic devices, as well as in Raman measurements of thermal transport in graphene and other two-dimensional materials.

  20. Combined effect of edge roughness and phonon scattering on the electronic properties of ultra scaled graphene nano-ribbons

    NASA Astrophysics Data System (ADS)

    Akhoondali, Hossein; Goharrizi, Arash Yazdanpanah; Sharifi, Mohammad Javad

    2014-11-01

    The effect of optical and acoustic phonon-scattering in the presence of line-edge-roughness (LER) on the electronic properties of ultra-scaled armchair graphene nano-ribbons (AGNRs) is investigated. Non-equilibrium Green's function formalism (NEGF) is employed using a Hamiltonian formed from tight bonding model with consideration of first and third nearest neighbors. The combined effect of phonons and line edge roughness on the transmission, transport gap, and conductance are studied for different roughness strengths and AGNR lengths. Results show edge roughness slightly reduces the onset of optical phonon emission, acoustic phonons reduce off-state conductance and optical phonons reduce on-state conductance. In both cases, the degree and behavior of reduction is totally dependent on the intensity of edge roughness. Also, in the longer AGNRs with high edge roughness intensity, phonons increase the transport gap.

  1. Electron-phonon interaction and scattering in Si and Ge: Implications for phonon engineering

    SciTech Connect

    Tandon, Nandan; Albrecht, J. D.; Ram-Mohan, L. R.

    2015-07-28

    We report ab-initio results for electron-phonon (e-ph) coupling and display the existence of a large variation in the coupling parameter as a function of electron and phonon dispersion. This variation is observed for all phonon modes in Si and Ge, and we show this for representative cases where the initial electron states are at the band gap edges. Using these e-ph matrix elements, which include all possible phonon modes and electron bands within a relevant energy range, we evaluate the imaginary part of the electron self-energy in order to obtain the associated scattering rates. The temperature dependence is seen through calculations of the scattering rates at 0 K and 300 K. The results provide a basis for understanding the impacts of phonon scattering vs. orientation and geometry in the design of devices, and in analysis of transport phenomena. This provides an additional tool for engineering the transfer of energy from carriers to the lattice.

  2. Preface to special topic: Selected articles from phononics 2013: The second international conference on phononic crystals/metamaterials, phonon transport and optomechanics, 2-7 June 2013, Sharm El-Sheikh, Egypt

    DOE PAGES

    Hussein, Mahmoud I.; El-Kady, Ihab; Li, Baowen; ...

    2014-12-31

    “Phononics” is an interdisciplinary branch of physics and engineering that deals with the behavior of phonons, and more broadly elastic and acoustic waves in similar context, and their manipulation in solids and/or fluids to benefit technological applications. Compared to resembling disciplines, such as electronics and photonics, phononics is a youthful field. It is growing at a remarkable rate, especially when viewed liberally with no limiting constraints on any particular length scale, discipline or application.

  3. Phonon waveguides for electromechanical circuits.

    PubMed

    Hatanaka, D; Mahboob, I; Onomitsu, K; Yamaguchi, H

    2014-07-01

    Nanoelectromechanical systems (NEMS), utilizing localized mechanical vibrations, have found application in sensors, signal processors and in the study of macroscopic quantum mechanics. The integration of multiple mechanical elements via electrical or optical means remains a challenge in the realization of NEMS circuits. Here, we develop a phonon waveguide using a one-dimensional array of suspended membranes that offers purely mechanical means to integrate isolated NEMS resonators. We demonstrate that the phonon waveguide can support and guide mechanical vibrations and that the periodic membrane arrangement also creates a phonon bandgap that enables control of the phonon propagation velocity. Furthermore, embedding a phonon cavity into the phonon waveguide allows mobile mechanical vibrations to be dynamically switched or transferred from the waveguide to the cavity, thereby illustrating the viability of waveguide-resonator coupling. These highly functional traits of the phonon waveguide architecture exhibit all the components necessary to permit the realization of all-phononic NEMS circuits.

  4. Forbidden phonon: Dynamical signature of bond symmetry breaking in the iron chalcogenides

    NASA Astrophysics Data System (ADS)

    Fobes, David M.; Zaliznyak, Igor A.; Tranquada, John M.; Xu, Zhijun; Gu, Genda; He, Xu-Gang; Ku, Wei; Zhao, Yang; Matsuda, Masaaki; Garlea, V. Ovidiu; Winn, Barry

    2016-09-01

    Investigation of the inelastic neutron scattering spectra in Fe1 +yTe1 -xSex near a signature wave vector Q =(1 ,0 ,0 ) for the bond-order wave (BOW) formation of parent compound Fe1 +yTe [D. Fobes et al., Phys. Rev. Lett. 112, 187202 (2014), 10.1103/PhysRevLett.112.187202] reveals an acoustic-phonon-like dispersion present in all structural phases. While a structural Bragg peak accompanies the mode in the low-temperature phase of Fe1 +yTe , it is absent in the high-temperature tetragonal phase, where Bragg scattering at this Q is forbidden by symmetry. Notably, this mode is also observed in superconducting FeTe0.55Se0.45 , where structural and magnetic transitions are suppressed, and no BOW has been observed. The presence of this "forbidden" phonon indicates that the lattice symmetry is dynamically or locally broken by magneto-orbital BOW fluctuations, which are strongly coupled to lattice in these materials.

  5. Electronic structure and electron-phonon coupling in TiH$_2$

    SciTech Connect

    Shanavas, Kavungal Veedu; Lindsay, Lucas R.; Parker, David S.

    2016-06-15

    Calculations using first principles methods and strong coupling theory are carried out to understand the electronic structure and superconductivity in cubic and tetragonal TiH$_2$. A large electronic density of states at the Fermi level in the cubic phase arises from Ti-$t_{2g}$ states and leads to a structural instability against tetragonal distortion at low temperatures. However, constraining the in-plane lattice constants diminishes the energy gain associated with the tetragonal distortion, allowing the cubic phase to be stable at low temperatures. Furthermore, calculated phonon dispersions show decoupled acoustic and optic modes arising from Ti and H vibrations, respectively and frequencies of optic modes to be rather high. The cubic phase has a large electron-phonon coupling parameter $\\lambda$ and critical temperature of several K. Contribution of the hydrogen sublattice to $\\lambda$ is found to be small in this material, which we understand from strong coupling theory to be due to the small H-$s$ DOS at the Fermi level and high energy of hydrogen modes at the tetrahedral sites.

  6. Electronic structure and electron-phonon coupling in TiH$$_2$$

    DOE PAGES

    Shanavas, Kavungal Veedu; Lindsay, Lucas R.; Parker, David S.

    2016-06-15

    Calculations using first principles methods and strong coupling theory are carried out to understand the electronic structure and superconductivity in cubic and tetragonal TiHmore » $$_2$$. A large electronic density of states at the Fermi level in the cubic phase arises from Ti-$$t_{2g}$$ states and leads to a structural instability against tetragonal distortion at low temperatures. However, constraining the in-plane lattice constants diminishes the energy gain associated with the tetragonal distortion, allowing the cubic phase to be stable at low temperatures. Furthermore, calculated phonon dispersions show decoupled acoustic and optic modes arising from Ti and H vibrations, respectively and frequencies of optic modes to be rather high. The cubic phase has a large electron-phonon coupling parameter $$\\lambda$$ and critical temperature of several K. Contribution of the hydrogen sublattice to $$\\lambda$$ is found to be small in this material, which we understand from strong coupling theory to be due to the small H-$s$ DOS at the Fermi level and high energy of hydrogen modes at the tetrahedral sites.« less

  7. Forbidden phonon: Dynamical signature of bond symmetry breaking in the iron chalcogenides

    DOE PAGES

    Fobes, David M.; Zaliznyak, Igor A.; Tranquada, John M.; ...

    2016-09-01

    Investigation of the inelastic neutron scattering spectra in Fe1+yTe1₋xSex near a signature wave vector Q=(1,0,0) for the bond-order wave (BOW) formation of parent compound Fe1+yTe reveals an acoustic-phonon-like dispersion present in all structural phases. While a structural Bragg peak accompanies the mode in the low-temperature phase of Fe1+yTe, it is absent in the high-temperature tetragonal phase, where Bragg scattering at this Q is forbidden by symmetry. Notably, this mode is also observed in superconducting FeTe0.55Se0.45, where structural and magnetic transitions are suppressed, and no BOW has been observed. Lastly, the presence of this “forbidden” phonon indicates that the lattice symmetrymore » is dynamically or locally broken by magneto-orbital BOW fluctuations, which are strongly coupled to lattice in these materials.« less

  8. Electronic structure and electron-phonon coupling in TiH2

    PubMed Central

    Shanavas, K. V.; Lindsay, L.; Parker, D. S.

    2016-01-01

    Calculations using first principles methods and strong coupling theory are carried out to understand the electronic structure and superconductivity in cubic and tetragonal TiH2. A large electronic density of states at the Fermi level in the cubic phase arises from Ti-t2g states and leads to a structural instability towards tetragonal distortion at low temperatures. However, constraining the in-plane lattice constants diminishes the energy gain associated with the tetragonal distortion, allowing the cubic phase to be stable at low temperatures. Calculated phonon dispersions show decoupled acoustic and optic modes arising from Ti and H vibrations, respectively, and frequencies of optic modes to be rather high. The cubic phase has a large electron-phonon coupling parameter λ and critical temperature of several K. Contribution of the hydrogen sublattice to λ is found to be small in this material, which we understand from strong coupling theory to be due to the small H-s DOS at the Fermi level and high energy of hydrogen modes at the tetrahedral sites. PMID:27302645

  9. Forbidden phonon: Dynamical signature of bond symmetry breaking in the iron chalcogenides

    SciTech Connect

    Fobes, David M.; Zaliznyak, Igor A.; Tranquada, John M.; Xu, Zhijun; Gu, Genda; He, Xu-Gang; Ku, Wei; Zhao, Yang; Matsuda, Masaaki; Garlea, V. Ovidiu; Winn, Barry

    2016-09-01

    Investigation of the inelastic neutron scattering spectra in Fe1+yTe1₋xSex near a signature wave vector Q=(1,0,0) for the bond-order wave (BOW) formation of parent compound Fe1+yTe reveals an acoustic-phonon-like dispersion present in all structural phases. While a structural Bragg peak accompanies the mode in the low-temperature phase of Fe1+yTe, it is absent in the high-temperature tetragonal phase, where Bragg scattering at this Q is forbidden by symmetry. Notably, this mode is also observed in superconducting FeTe0.55Se0.45, where structural and magnetic transitions are suppressed, and no BOW has been observed. Lastly, the presence of this “forbidden” phonon indicates that the lattice symmetry is dynamically or locally broken by magneto-orbital BOW fluctuations, which are strongly coupled to lattice in these materials.

  10. Surface Phonons and Polaritons.

    DTIC Science & Technology

    1976-01-01

    for an impurity in the surface of a crystal could be observed in the one phonon cross section for the resonant absorption or e.ission of ,—rays by...localized at the surface. The w5 — dependence has a simple physical origin. It is well known that the cross section for scattering of bulk phonons by a...propagate. In Section II of the present Chapter we present the theory underlying the surface induced vibrational properties of crystals which we have

  11. Effects of ternary mixed crystal and size on optical phonons in wurtzite nitride core-shell nanowires

    SciTech Connect

    Li, J.; Guan, J. Y.; Zhang, S. F.; Ban, S. L.; Qu, Y.

    2014-04-21

    Within the framework of dielectric continuum and Loudon's uniaxial crystal models, existence conditions dependent on components and frequencies for optical phonons in wurtzite nitride core-shell nanowires (CSNWs) are discussed to obtain dispersion relations and electrostatic potentials of optical phonons in In{sub x}Ga{sub 1−x}N/GaN CSNWs. The results show that there may be four types of optical phonons in In{sub x}Ga{sub 1−x}N/GaN CSNWs for a given ternary mixed crystal (TMC) component due to the phonon dispersion anisotropy. This property is analogous to wurtzite planar heterojunctions. Among the optical phonons, there are two types of quasi-confined optical (QCO) phonons (named, respectively, as QCO-A and QCO-B), one type of interface (IF) phonons and propagating (PR) phonons existing in certain component and frequency domains while the dispersion relations and electrostatic potentials of same type of optical phonons vary with components. Furthermore, the size effect on optical phonons in CSNWs is also discussed. The dispersion relations of IF and QCO-A are independent of the boundary location of CSNWs. Meanwhile, dispersion relations and electrostatic potentials of QCO-B and PR phonons vary obviously with size, especially, when the ratio of a core radius to a shell radius is small, and dispersion relation curves of PR phonons appear to be close to each other, whereas, this phenomenon disappears when the ratio becomes large. Based on our conclusions, one can further discuss photoelectric properties in nitride CSNWs consisting of TMCs associated with optical phonons.

  12. Light scattering from acoustic vibrational modes in confined structures

    NASA Astrophysics Data System (ADS)

    Bandhu, Rudra Shyam

    The acoustic vibrational modes and their light scattering intensities in confined structures such as supported films, double layer free-standing membrane and sub-micron sized wires on a free-standing membrane have been studied using Brillouin Light Scattering (BLS). Standing wave type acoustic phonons were recently observed in supported thin films of silicon oxy-nitride. We build upon this finding to study the acoustic modes in thin zinc selenide (ZnSe) films on gallium arsenide (GaAs). The surprising behaviour of the Brillouin intensities of the standing wave modes in ZnSe are explained in terms of interference of the elasto-optic scattering amplitudes from the film and substrate. Numerical calculations of the scattering cross-section, which takes into account ripple and elasto-optic scattering mechanism, agrees well with the experimental data. Light scattering studies of standing wave type modes in free-standing polymethyl methacrylate (PMMA) layer on Si3N4 were carried out. In these bilayer structures PMMA is much softer than Si3N 4, a property that leads to confinement of low frequency modes associated with the PMMA layer to within its boundaries. In addition, the flexural and the dilatational modes from the Si3N4 layer are observed and are found to hybridize with the standing wave modes from the PMMA layer. Our study of phonon modes in PMMA wires supported on a free-standing Si3N4 membrane extends our work on free-standing double layer membranes. In recent years there is much interest in the study of phonon modes in nano-scale structures such as wires or dots. Although much theoretical work has been carried out in this direction, no experiments exist that explore the dispersion of the phonon modes in such structures. Brillouin Light scattering is ideally suited for studying phonons in such reduced dimensions and our work represents the first effort in this direction. The spectra reveal modes which are quantized both along the width, as well along the thickness

  13. Design and Optimization of Omnidirectional Band Gap for One-Dimensional Periodic and Quasiperiodic Phononic Heterostructures

    NASA Astrophysics Data System (ADS)

    Chen, Zhao-Jiang

    2015-01-01

    A new kind of one-dimensional multilayer phononic heterostructure is constructed to obtain a broad acoustic omnidirectional reflection (ODR) band. The heterostructure is formed by combining finite periodic phononic crystals (PnCs) and Fibonacci (or Thue—Morse) quasiperiodic PnCs. From the numerical results performed by the transfer matrix method, it is found that the ODR bands can be enlarged obviously by using the combination of periodic and quasi-periodic PnCs. Moreover, an application of particle swarm optimization in designing and optimizing acoustic ODR bands is reported. With regards to different thickness ratios and periodic numbers in the heterostructure, we give some optimization examples and finally achieve phononic heterostructure with a very broad ODR bandwidth. The result provides a new approach to achieve broad acoustic ODR bandwidth, and will be applied in design of omnidirectional acoustic mirrors.

  14. Weak coupling of pseudoacoustic phonons and magnon dynamics in the incommensurate spin-ladder compound Sr14Cu24O41

    SciTech Connect

    Chen, Xi; Bansal, Dipanshu; Sullivan, Sean; Abernathy, Douglas L.; Aczel, Adam A.; Zhou, Jianshi; Delaire, Olivier A.; Shi, Li

    2016-10-21

    Intriguing lattice dynamics have been predicted for aperiodic crystals that contain incommensurate substructures. Here we report inelastic neutron scattering measurements of phonon and magnon dispersions in Sr14Cu24O41, which contains incommensurate one-dimensional (1D) chain and two-dimensional (2D) ladder substructures. Two distinct pseudoacoustic phonon modes, corresponding to the sliding motion of one sublattice against the other, are observed for atomic motions polarized along the incommensurate axis. In the long wavelength limit, it is found that the sliding mode shows a remarkably small energy gap of 1.7–1.9 meV, indicating very weak interactions between the two incommensurate sublattices. The measurements also reveal a gapped and steep linear magnon dispersion of the ladder sublattice. The high group velocity of this magnon branch and weak coupling with acoustic and pseudoacoustic phonons can explain the large magnon thermal conductivity in Sr14Cu24O41 crystals. In addition, the magnon specific heat is determined from the measured total specific heat and phonon density of states and exhibits a Schottky anomaly due to gapped magnon modes of the spin chains. Furthermore, these findings offer new insights into the phonon and magnon dynamics and thermal transport properties of incommensurate magnetic crystals that contain low-dimensional substructures.

  15. Phonons of the anomalous element cerium

    PubMed Central

    Krisch, Michael; Farber, D. L.; Xu, R.; Antonangeli, Daniele; Aracne, C. M.; Beraud, Alexandre; Chiang, Tai-Chang; Zarestky, J.; Kim, Duck Young; Isaev, Eyvaz I.; Ahuja, Rajeev; Johansson, Börje

    2011-01-01

    Many physical and chemical properties of the light rare-earths and actinides are governed by the active role of f electrons, and despite intensive efforts the details of the mechanisms of phase stability and transformation are not fully understood. A prominent example which has attracted a lot of interest, both experimentally and theoretically over the years is the isostructural γ - α transition in cerium. We have determined by inelastic X-ray scattering, the complete phonon dispersion scheme of elemental cerium across the γ → α transition, and compared it with theoretical results using ab initio lattice dynamics. Several phonon branches show strong changes in the dispersion shape, indicating large modifications in the interactions between phonons and conduction electrons. This is reflected as well by the lattice Grüneisen parameters, particularly around the X point. We derive a vibrational entropy change , illustrating the importance of the lattice contribution to the transition. Additionally, we compare first principles calculations with the experiments to shed light on the mechanism underlying the isostructural volume collapse in cerium under pressure. PMID:21597000

  16. Electron–phonon coupling in hybrid lead halide perovskites

    PubMed Central

    Wright, Adam D.; Verdi, Carla; Milot, Rebecca L.; Eperon, Giles E.; Pérez-Osorio, Miguel A.; Snaith, Henry J.; Giustino, Feliciano; Johnston, Michael B.; Herz, Laura M.

    2016-01-01

    Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH2)2PbI3, HC(NH2)2PbBr3, CH3NH3PbI3 and CH3NH3PbBr3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron–phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ∼40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites. PMID:27225329

  17. Electron-phonon coupling in hybrid lead halide perovskites

    NASA Astrophysics Data System (ADS)

    Wright, Adam D.; Verdi, Carla; Milot, Rebecca L.; Eperon, Giles E.; Pérez-Osorio, Miguel A.; Snaith, Henry J.; Giustino, Feliciano; Johnston, Michael B.; Herz, Laura M.

    2016-05-01

    Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH2)2PbI3, HC(NH2)2PbBr3, CH3NH3PbI3 and CH3NH3PbBr3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron-phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ~40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites.

  18. Electron-phonon coupling in hybrid lead halide perovskites.

    PubMed

    Wright, Adam D; Verdi, Carla; Milot, Rebecca L; Eperon, Giles E; Pérez-Osorio, Miguel A; Snaith, Henry J; Giustino, Feliciano; Johnston, Michael B; Herz, Laura M

    2016-05-26

    Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH2)2PbI3, HC(NH2)2PbBr3, CH3NH3PbI3 and CH3NH3PbBr3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron-phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ∼40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites.

  19. Electron-phonon interactions and the intrinsic electrical resistivity of graphene.

    PubMed

    Park, Cheol-Hwan; Bonini, Nicola; Sohier, Thibault; Samsonidze, Georgy; Kozinsky, Boris; Calandra, Matteo; Mauri, Francesco; Marzari, Nicola

    2014-03-12

    We present a first-principles study of the temperature- and density-dependent intrinsic electrical resistivity of graphene. We use density-functional theory and density-functional perturbation theory together with very accurate Wannier interpolations to compute all electronic and vibrational properties and electron-phonon coupling matrix elements; the phonon-limited resistivity is then calculated within a Boltzmann-transport approach. An effective tight-binding model, validated against first-principles results, is also used to study the role of electron-electron interactions at the level of many-body perturbation theory. The results found are in excellent agreement with recent experimental data on graphene samples at high carrier densities and elucidate the role of the different phonon modes in limiting electron mobility. Moreover, we find that the resistivity arising from scattering with transverse acoustic phonons is 2.5 times higher than that from longitudinal acoustic phonons. Last, high-energy, optical, and zone-boundary phonons contribute as much as acoustic phonons to the intrinsic electrical resistivity even at room temperature and become dominant at higher temperatures.

  20. Phonon-lifetimes in demixing systems

    NASA Astrophysics Data System (ADS)

    Davaasambuu, J.; Güthoff, F.; Petri, M.; Hradil, K.; Schober, H.; Ollivier, J.; Eckold, G.

    2012-06-01

    The dynamics of silver-alkali halide mixed single crystals (AgxNa1-xBr, x = 0.23, 0.35, 0.40 and 0.70) were studied by inelastic neutron scattering during the process of spinodal decomposition. Using the thermal three-axes spectrometer PUMA as well as the time-of-flight spectrometer IN5, the time evolution of phonons was observed in time-resolved, stroboscopic measurements. Complementary to the study of long wavelength acoustic phonons, as studied previously, we extended these investigations to Brillouin-zone boundary modes that are particularly sensitive to variations of the local structure. Starting from the homogeneous mixed phase the behaviour of these modes during demixing is observed in real-time. A simple dynamical model based on local structure variants helps to interpret the results. It is shown that the phonon lifetimes vary strongly during the phase separation and increase drastically during the coarsening process. Up to a critical size of precipitates of about 10 nm, zone-boundary modes are found to be strongly damped, while beyond the line widths are reduced to the experimental resolution. This finding leads to the conclusion that the typical mean free path of these modes is of the order of 10 nm, which corresponds to 20 unit cells.

  1. ThermoPhonon

    SciTech Connect

    Zarkevich, Nikolai

    2014-11-24

    ThermoPhonon is a stand-alone code, which can be integrated into other software packages. Typically, it is used together with a density functional theory (DFT) code (such as VASP, Wien2k, AbInit, SIESTA) and a phonon code (such as Phonopy or Phon). The workflow is the following. Molecular dynamics (MD) in a supercell at a given temperature T is performed using another code. After sufficient equilibration, the output in the form of atomic positions and forces for a large number of selected MD steps is recorded into a file. If needed, one can modify this file by applying additional constraints, such as enforced crystal symmetry or subtracted motion of the center of mass. ThermoPhonon reads the file with atomic positions and forces and writes a new file with the force constants. Force constants can be used by another code (such as Phonopy or Phon) to produce phonon spectrum for plotting, in the assumption of known equilibrium atomic positions provided in a separate file.

  2. Phonons, Atoms, and Waves

    ERIC Educational Resources Information Center

    Reid, John S.

    1977-01-01

    Discussed are how the thermal vibrations of a solid are described in terms of lattice waves, how these waves interact with other waves, or with themselves, and how one is led from such a description in terms of waves to the concept of a phonon. (Author/MA)

  3. Laser-enabled experimental wavefield reconstruction in two-dimensional phononic crystals

    NASA Astrophysics Data System (ADS)

    Celli, Paolo; Gonella, Stefano

    2014-01-01

    During the past two decades, noteworthy experimental investigations have been conducted on wave propagation in phononic crystals, with special emphasis on crystals for acoustic wave control, consisting of the repetition of cylindrical or spherical elements in a fluid medium. On the other hand, the experimental characterization of the elastic wave phenomena observed in the solid microstructure of phononic crystals designed for elastic wave control has been quite sparse and limited in scope. The related literature focuses mostly on steady-state analyses that aim at highlighting filtering properties, and are limited to out-of-plane measurements. The scope of this work is to address these limitations and provide a detailed experimental characterization of the transient wave phenomena observed in the cores of lattice-like phononic crystals. This is achieved using a 3D Scanning Laser Vibrometer, which allows measuring the in-plane velocity of material points belonging to the lattice topology. This approach is tested against the benchmark case of a regular honeycomb lattice. Specifically, the objective is to demonstrate the directional and dispersive nature of the S-mode at relatively low frequencies and characterize the P-mode below and above its veering frequency. The experimental results are compared against numerical simulations and unit cell Bloch analysis to highlight similarities and differences between the true response of finite crystals and the infinite lattice approximation. This study also intends to highlight the advantages of three-dimensional laser vibrometry as a tool for the characterization of complex structural materials, while carefully exposing some limitations of this methodology.

  4. Phonon transport properties of two-dimensional group-IV materials from ab initio calculations

    NASA Astrophysics Data System (ADS)

    Peng, Bo; Zhang, Hao; Shao, Hezhu; Xu, Yuanfeng; Ni, Gang; Zhang, Rongjun; Zhu, Heyuan

    2016-12-01

    It has been argued that stanene has lowest lattice thermal conductivity among two-dimensional (2D) group-IV materials because of its largest atomic mass, weakest interatomic bonding, and enhanced ZA phonon scattering due to the breaking of an out-of-plane symmetry selection rule. However, we show that, although the lattice thermal conductivity κ for graphene, silicene, and germanene decreases monotonically with decreasing Debye temperature, unexpected higher κ is observed in stanene. By enforcing all the invariance conditions in 2D materials and including Ge 3 d and Sn 4 d electrons as valence electrons for germanene and stanene, respectively, the lattice dynamics in these materials are accurately described. A large acoustic-optical gap and the bunching of the acoustic-phonon branches significantly reduce phonon scattering in stanene, leading to higher thermal conductivity than germanene. The vibrational origin of the acoustic-optical gap can be attributed to the buckled structure. Interestingly, a buckled system has two competing influences on phonon transport: the breaking of the symmetry selection rule leads to reduced thermal conductivity, and the enlarging of the acoustic-optical gap results in enhanced thermal conductivity. The size dependence of thermal conductivity is investigated as well. In nanoribbons, the κ of silicene, germanene, and stanene is much less sensitive to size effect due to their short intrinsic phonon mean-free paths. This work sheds light on the nature of phonon transport in buckled 2D materials.

  5. Stability analysis and investigation of higher order Schrödinger equation for strongly dispersive ion-acoustic wave in plasma

    NASA Astrophysics Data System (ADS)

    Gogoi, R.; Kalita, L.; Devi, N.

    2010-02-01

    Much interest was shown towards the studies on nonlinear stability in the late sixties. Plasma instabilities play an important role in plasma dynamics. More attention has been given towards stability analysis after recognizing that they are one of the principal obstacles in the way of a successful resolution of the problem of controlled thermonuclear fusion. Nonlinearity and dispersion are the two important characteristics of plasma instabilities. Instabilities and nonlinearity are the two important and interrelated terms. In our present work, the continuity and momentum equations for both ions and electrons together with the Poisson equation are considered as cold plasma model. Then we have adopted the modified reductive perturbation technique (MRPT) from Demiray [1] to derive the higher order equation of the Nonlinear Schrödinger equation (NLSE). In this work, detailed mathematical expressions and calculations are done to investigate the changing character of the modulation of ion acoustic plasma wave through our derived equation. Thus we have extended the application of MRPT to derive the higher order equation. Both progressive wave solutions as well as steady state solutions are derived and they are plotted for different plasma parameters to observe dark/bright solitons. Interesting structures are found to exist for different plasma parameters.

  6. Phonon properties of graphene derived from molecular dynamics simulations

    PubMed Central

    Koukaras, Emmanuel N.; Kalosakas, George; Galiotis, Costas; Papagelis, Konstantinos

    2015-01-01

    A method that utilises atomic trajectories and velocities from molecular dynamics simulations has been suitably adapted and employed for the implicit calculation of the phonon dispersion curves of graphene. Classical potentials widely used in the literature were employed. Their performance was assessed for each individual phonon branch and the overall phonon dispersion, using available inelastic x-ray scattering data. The method is promising for systems with large scale periodicity, accounts for anharmonic effects and non-bonding interactions with a general environment, and it is applicable under finite temperatures. The temperature dependence of the phonon dispersion curves has been examined with emphasis on the doubly degenerate Raman active Γ-E2g phonon at the zone centre, where experimental results are available. The potentials used show diverse behaviour. The Tersoff-2010 potential exhibits the most systematic and physically sound behaviour in this regard, and gives a first-order temperature coefficient of χ = −0.05 cm−1/K for the Γ-E2g shift in agreement with reported experimental values. PMID:26316252

  7. Phonon quarticity induced by changes in phonon-tracked hybridization during lattice expansion and its stabilization of rutile TiO2

    DOE PAGES

    Lan, Tian; Li, Chen W.; Hellman, O.; ...

    2015-08-11

    Although the rutile structure of TiO2 is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly predicting a structural collapse at temperatures well below 1000 K. In this paper, inelastic neutron scattering was used to measure the temperature dependence of the phonon density of states (DOS) of rutile TiO2 from 300 to 1373 K. Surprisingly, these anomalous acoustic phonons were found to increase in frequency with temperature. First-principles calculations showed that with lattice expansion, the potentials for the anomalous acoustic phonons transform from quadratic to quartic, stabilizingmore » the rutile phase at high temperatures. In these modes, the vibrational displacements of adjacent Ti and O atoms cause variations in hybridization of 3d electrons of Ti and 2p electrons of O atoms. Finally, with thermal expansion, the energy variation in this “phonon-tracked hybridization” flattens the bottom of the interatomic potential well between Ti and O atoms, and induces a quarticity in the phonon potential.« less

  8. Coulomb and electron-phonon interactions in metals

    NASA Astrophysics Data System (ADS)

    Tupitsyn, Igor S.; Mishchenko, Andrey S.; Nagaosa, Naoto; Prokof'ev, Nikolay

    2016-10-01

    An accurate and consistent theory of phonons in metals requires that all long-range Coulomb interactions between charged particles (electrons and ions) be treated on equal footing. So far, all attempts to deal with this nonperturbative system were relying on uncontrolled approximations in the absence of small parameters. In this paper, we develop the diagrammatic Monte Carlo approach for a two-component Coulomb system that obtains the solution to this fundamental problem in an approximation-free way by computing vertex corrections from higher-order skeleton graphs. The feasibility of the method is demonstrated by calculating the spectrum of longitudinal acoustic phonons in a simple cubic lattice, determining their sound velocity, and obtaining the phonon spectral densities by analytic continuation of the Matsubara-Green's functions. Final results are checked against the lowest-order fully self-consistent G W approximation in both adiabatic and nonadiabatic regimes.

  9. A GaAs phononic crystal with shallow noncylindrical holes.

    PubMed

    Petrus, Joseph A; Mathew, Reuble; Stotz, James A H

    2014-02-01

    A square lattice of shallow, noncylindrical holes in GaAs is shown to act as a phononic crystal (PnC) reflector. The holes are produced by wet-etching a GaAs substrate using a citric acid:H2O2 etching procedure and a photolithographed array pattern. Although nonuniform and asymmetric etch rates limit the depth and shape of the phononic crystal holes, the matrix acts as a PnC, as demonstrated by insertion loss measurements together with interferometric imaging of surface acoustic waves propagating on the GaAs surface. The measured vertical displacement induced by surface phonons compares favorably with finite-difference time-domain simulations of a PnC with rounded-square holes.

  10. Phononic crystal plate with hollow pillars connected by thin bars

    NASA Astrophysics Data System (ADS)

    Jin, Yabin; Pennec, Yan; Pan, Yongdong; Djafari-Rouhani, Bahram

    2017-01-01

    A new type of phononic crystal plate consisting of hollow pillars on a bar-connected plate is proposed. With respect to usual pillar based phononic crystal plates, the Bragg band gap can be tuned to be much wider and extended to a sub-wavelength region, and the low frequency gap can be moved to an extremely low frequency range. Such a structure can generate quadrapolar, hexapolar and octopolar whispering-gallery modes (WGMs) inside the band gaps with very high confinement and quality factors. By filling the hollow pillars with a liquid, these WGMs, together with additional localized compressional and solid-liquid coupling modes, can be tuned either by varying the inner radius of the pillars or controlling the height of the liquid. We discuss some possible functionalities of these phononic crystals for the purpose of sensing the acoustic properties of liquids, multiplexer and wireless communication.

  11. Phonon modes at the 2H-NbSe2 surface observed by grazing incidence inelastic x-ray scattering.

    PubMed

    Murphy, B M; Requardt, H; Stettner, J; Serrano, J; Krisch, M; Müller, M; Press, W

    2005-12-16

    We have determined the dispersion of acoustic and optical surface phonon modes 2H-NbSe2 at the by inelastic x-ray scattering under grazing incidence conditions. Already, at room temperature, an anomaly is observed close to the charge density wave -vector position located at about one-third along the Gamma-M direction of the Brillouin zone. Our results indicate that the anomaly for the surface mode occurs at a lower energy than that measured in bulk sensitive geometry in the same experiment, showing evidence of a modified behavior in the uppermost layers. We demonstrate that inelastic x-ray scattering in grazing incidence conditions provides a unique tool to selectively study either surface or bulk lattice dynamics in a single experiment.

  12. Edge waves and resonances in two-dimensional phononic crystal plates

    NASA Astrophysics Data System (ADS)

    Hsu, Jin-Chen; Hsu, Chih-Hsun

    2015-05-01

    We present a numerical study on phononic band gaps and resonances occurring at the edge of a semi-infinite two-dimensional (2D) phononic crystal plate. The edge supports localized edge waves coupling to evanescent phononic plate modes that decay exponentially into the semi-infinite phononic crystal plate. The band-gap range and the number of edge-wave eigenmodes can be tailored by tuning the distance between the edge and the semi-infinite 2D phononic lattice. As a result, a phononic band gap for simultaneous edge waves and plate waves is created, and phononic cavities beside the edge can be built to support high-frequency edge resonances. We design an L3 edge cavity and analyze its resonance characteristics. Based on the band gap, high quality factor and strong confinement of resonant edge modes are achieved. The results enable enhanced control over acoustic energy flow in phononic crystal plates, which can be used in designing micro and nanoscale resonant devices and coupling of edge resonances to other types of phononic or photonic crystal cavities.

  13. Hole-interface optical phonon relaxation rates with valence band-mixing effects

    NASA Astrophysics Data System (ADS)

    Kim, Cheol-Hoi

    2004-05-01

    We theoretically investigate the hole-interface optical phonon scattering rates for a InGaAs-AlGaAs quantum well structure, taking into account the valence-band mixing. The dispersion relation and the electrostatic potentials for interface optical phonon modes are obtained based on the macroscopic dielectric continuum model. For the hole dispersion relation, the Luttinger-Kohn Hamiltonian is used. The hole-interface optical phonon interaction is evaluated by the Fermi's golden rule taking into account the Bloch overlap factor. Our results show that the hole-interface phonon scattering rates within the parabolic band approximation are different from those including valence band mixing effects. Especially, in the low energy region, the hole-interface phonon scattering rates within the parabolic band approximation are overestimated very significantly.

  14. Phonons and thermal transport in graphene and graphene-based materials

    NASA Astrophysics Data System (ADS)

    Nika, Denis L.; Balandin, Alexander A.

    2017-03-01

    A discovery of the unusual thermal properties of graphene stimulated experimental, theoretical and computational research directed at understanding phonon transport and thermal conduction in two-dimensional material systems. We provide a critical review of recent results in the graphene thermal field focusing on phonon dispersion, specific heat, thermal conductivity, and comparison of different models and computational approaches. The correlation between the phonon spectrum in graphene-based materials and the heat conduction properties is analyzed in details. The effects of the atomic plane rotations in bilayer graphene, isotope engineering, and relative contributions of different phonon dispersion branches are discussed. For readers’ convenience, the summaries of main experimental and theoretical results on thermal conductivity as well as phonon mode contributions to thermal transport are provided in the form of comprehensive annotated tables.

  15. Gallium nitride electro-acoustic devices and acoustic metamaterials

    NASA Astrophysics Data System (ADS)

    Rais-Zadeh, Mina

    2016-05-01

    Gallium nitride (GaN) being one of a few piezoelectric semiconductors with low acoustic loss is a perfect material for electro-acoustic applications. Interactions of electrons and phonons are facilitated by the piezoelectric effect in addition to the deformation coupling in GaN, a property that can be used to implement a variety of very interesting devices and metamaterials, such as resonant transistors, acoustic amplifiers, circulators, and couplers. This talk covers theoretical basis of such devices and overviews recent advances in this technology.

  16. Phonon anharmonicity and negative thermal expansion in SnSe

    SciTech Connect

    Bansal, Dipanshu; Hong, Jiawang; Li, Chen W.; May, Andrew F.; Porter, Wallace; Hu, Michael Y.; Abernathy, Douglas L.; Delaire, Olivier

    2016-08-09

    In this paper, the anharmonic phonon properties of SnSe in the Pnma phase were investigated with a combination of experiments and first-principles simulations. Using inelastic neutron scattering (INS) and nuclear resonant inelastic X-ray scattering (NRIXS), we have measured the phonon dispersions and density of states (DOS) and their temperature dependence, which revealed a strong, inhomogeneous shift and broadening of the spectrum on warming. First-principles simulations were performed to rationalize these measurements, and to explain the previously reported anisotropic thermal expansion, in particular the negative thermal expansion within the Sn-Se bilayers. Including the anisotropic strain dependence of the phonon free energy, in addition to the electronic ground state energy, is essential to reproduce the negative thermal expansion. From the phonon DOS obtained with INS and additional calorimetry measurements, we quantify the harmonic, dilational, and anharmonic components of the phonon entropy, heat capacity, and free energy. Finally, the origin of the anharmonic phonon thermodynamics is linked to the electronic structure.

  17. Phonon anharmonicity and negative thermal expansion in SnSe

    DOE PAGES

    Bansal, Dipanshu; Hong, Jiawang; Li, Chen W.; ...

    2016-08-09

    In this paper, the anharmonic phonon properties of SnSe in the Pnma phase were investigated with a combination of experiments and first-principles simulations. Using inelastic neutron scattering (INS) and nuclear resonant inelastic X-ray scattering (NRIXS), we have measured the phonon dispersions and density of states (DOS) and their temperature dependence, which revealed a strong, inhomogeneous shift and broadening of the spectrum on warming. First-principles simulations were performed to rationalize these measurements, and to explain the previously reported anisotropic thermal expansion, in particular the negative thermal expansion within the Sn-Se bilayers. Including the anisotropic strain dependence of the phonon free energy,more » in addition to the electronic ground state energy, is essential to reproduce the negative thermal expansion. From the phonon DOS obtained with INS and additional calorimetry measurements, we quantify the harmonic, dilational, and anharmonic components of the phonon entropy, heat capacity, and free energy. Finally, the origin of the anharmonic phonon thermodynamics is linked to the electronic structure.« less

  18. Orbitally-driven giant phonon anharmonicity in SnSe

    SciTech Connect

    Li, Chen W.; Hong, Jiawang; May, Andrew F.; Bansal, Dipanshu; Chi, Songxue; Hong, Tao; Ehlers, Georg; Delaire, Olivier A.

    2015-10-19

    We understand that elementary excitations and their couplings in condensed matter systems is critical to develop better energy-conversion devices. In thermoelectric materials, the heat-to-electricity conversion efficiency is directly improved by suppressing the propagation of phonon quasiparticles responsible for macroscopic thermal transport. The material with the current record for thermoelectric conversion efficiency, SnSe, achieves an ultra-low thermal conductivity, but the mechanism enabling this strong phonon scattering remains largely unknown. Using inelastic neutron scattering measurements and first-principles simulations, we mapped the four-dimensional phonon dispersion surfaces of SnSe, and revealed the origin of ionic-potential anharmonicity responsible for the unique properties of SnSe. We show that the giant phonon scattering arises from an unstable electronic structure, with orbital interactions leading to a ferroelectric-like lattice instability. Our results provide a microscopic picture connecting electronic structure and phonon anharmonicity in SnSe, and offers precious insights on how electron-phonon and phononphonon interactions may lead to the realization of ultra-low thermal conductivity.

  19. Orbitally-driven giant phonon anharmonicity in SnSe

    DOE PAGES

    Li, Chen W.; Hong, Jiawang; May, Andrew F.; ...

    2015-10-19

    We understand that elementary excitations and their couplings in condensed matter systems is critical to develop better energy-conversion devices. In thermoelectric materials, the heat-to-electricity conversion efficiency is directly improved by suppressing the propagation of phonon quasiparticles responsible for macroscopic thermal transport. The material with the current record for thermoelectric conversion efficiency, SnSe, achieves an ultra-low thermal conductivity, but the mechanism enabling this strong phonon scattering remains largely unknown. Using inelastic neutron scattering measurements and first-principles simulations, we mapped the four-dimensional phonon dispersion surfaces of SnSe, and revealed the origin of ionic-potential anharmonicity responsible for the unique properties of SnSe. Wemore » show that the giant phonon scattering arises from an unstable electronic structure, with orbital interactions leading to a ferroelectric-like lattice instability. Our results provide a microscopic picture connecting electronic structure and phonon anharmonicity in SnSe, and offers precious insights on how electron-phonon and phononphonon interactions may lead to the realization of ultra-low thermal conductivity.« less

  20. Phonon anharmonicity and negative thermal expansion in SnSe

    NASA Astrophysics Data System (ADS)

    Bansal, Dipanshu; Hong, Jiawang; Li, Chen W.; May, Andrew F.; Porter, Wallace; Hu, Michael Y.; Abernathy, Douglas L.; Delaire, Olivier

    2016-08-01

    The anharmonic phonon properties of SnSe in the P n m a phase were investigated with a combination of experiments and first-principles simulations. Using inelastic neutron scattering (INS) and nuclear resonant inelastic X-ray scattering (NRIXS), we have measured the phonon dispersions and density of states (DOS) and their temperature dependence, which revealed a strong, inhomogeneous shift and broadening of the spectrum on warming. First-principles simulations were performed to rationalize these measurements, and to explain the previously reported anisotropic thermal expansion, in particular the negative thermal expansion within the Sn-Se bilayers. Including the anisotropic strain dependence of the phonon free energy, in addition to the electronic ground state energy, is essential to reproduce the negative thermal expansion. From the phonon DOS obtained with INS and additional calorimetry measurements, we quantify the harmonic, dilational, and anharmonic components of the phonon entropy, heat capacity, and free energy. The origin of the anharmonic phonon thermodynamics is linked to the electronic structure.

  1. Shear surface waves in phononic crystals.

    PubMed

    Kutsenko, A A; Shuvalov, A L

    2013-02-01

    The existence of shear horizontal (SH) surface waves in two-dimensional periodic phononic crystals with an asymmetric depth-dependent profile is theoretically reported. Examples of dispersion spectra with bandgaps for subsonic and supersonic SH surface waves are demonstrated. The link between the effective (quasistatic) speeds of the SH bulk and surface waves is established. Calculation and analysis is based on the integral form of a projector on the subspace of evanescent modes which means no need for their explicit finding. This method can be extended to the vector waves and the three-dimensional case.

  2. Temperature induced phonon behaviour in germanium selenide thin films probed by Raman spectroscopy

    NASA Astrophysics Data System (ADS)

    Taube, A.; Łapińska, A.; Judek, J.; Wochtman, N.; Zdrojek, M.

    2016-08-01

    Here we report a detailed study of temperature-dependent phonon properties of exfoliated germanium selenide thin films (several tens of nanometers thick) probed by Raman spectroscopy in the 70-350 K temperature range. The temperature-dependent behavior of the positions and widths of the Raman modes was nonlinear. We concluded that the observed effects arise from anharmonic phonon-phonon interactions and are explained by the phenomenon of optical phonon decay into acoustic phonons. At temperatures above 200 K, the position of the Raman modes tended to be linearly dependent, and the first order temperature coefficients χ were  -0.0277, -0.0197 and  -0.031 cm-1 K-1 for B 3g , A g(1) and A g(2) modes, respectively.

  3. Yoctocalorimetry: phonon counting in nanostructures

    NASA Astrophysics Data System (ADS)

    Roukes, M. L.

    1999-03-01

    It appears feasible with nanostructures to perform calorimetry at the level of individual thermal phonons. Here I outline an approach employing monocrystalline mesoscopic insulators, which can now be patterned from semiconductor heterostructures into complex geometries with full, three-dimensional relief. Successive application of these techniques also enables definition of integrated nanoscale thermal transducers; coupling these to a dc SQUID readout yields the requisite energy sensitivity and temporal resolution with minimal back action. The prospect of phonon counting opens intriguing experimental possibilities with analogies in quantum optics. These include fluctuation-based phonon spectroscopy, phonon shot noise in the energy relaxation of nanoscale systems, and quantum statistical phenomena such as phonon bunching and anticorrelated electron-phonon exchange.

  4. Thermal characterization of nanoscale phononic crystals using supercell lattice dynamics

    NASA Astrophysics Data System (ADS)

    Davis, Bruce L.; Hussein, Mahmoud I.

    2011-12-01

    The concept of a phononic crystal can in principle be realized at the nanoscale whenever the conditions for coherent phonon transport exist. Under such conditions, the dispersion characteristics of both the constitutive material lattice (defined by a primitive cell) and the phononic crystal lattice (defined by a supercell) contribute to the value of the thermal conductivity. It is therefore necessary in this emerging class of phononic materials to treat the lattice dynamics at both periodicity levels. Here we demonstrate the utility of using supercell lattice dynamics to investigate the thermal transport behavior of three-dimensional nanoscale phononic crystals formed from silicon and cubic voids of vacuum. The periodicity of the voids follows a simple cubic arrangement with a lattice constant that is around an order of magnitude larger than that of the bulk crystalline silicon primitive cell. We consider an atomic-scale supercell which incorporates all the details of the silicon atomic locations and the void geometry. For this supercell, we compute the phonon band structure and subsequently predict the thermal conductivity following the Callaway-Holland model. Our findings dictate that for an analysis based on supercell lattice dynamics to be representative of the properties of the underlying lattice model, a minimum supercell size is needed along with a minimum wave vector sampling resolution. Below these minimum values, a thermal conductivity prediction of a bulk material based on a supercell will not adequately recover the value obtained based on a primitive cell. Furthermore, our results show that for the relatively small voids and void spacings we consider (where boundary scattering is dominant), dispersion at the phononic crystal unit cell level plays a noticeable role in determining the thermal conductivity.

  5. Acoustic neuroma

    MedlinePlus

    Vestibular schwannoma; Tumor - acoustic; Cerebellopontine angle tumor; Angle tumor; Hearing loss - acoustic; Tinnitus - acoustic ... Acoustic neuromas have been linked with the genetic disorder neurofibromatosis type 2 (NF2). Acoustic neuromas are uncommon.

  6. Hypersonic acoustic excitations in binary colloidal crystals: big versus small hard sphere control.

    PubMed

    Tommaseo, G; Petekidis, G; Steffen, W; Fytas, G; Schofield, A B; Stefanou, N

    2007-01-07

    The phononic band structure of two binary colloidal crystals, at hypersonic frequencies, is studied by means of Brillouin light scattering and analyzed in conjunction with corresponding dispersion diagrams of the single colloidal crystals of the constituent particles. Besides the acoustic band of the average medium, the authors' results show the existence of narrow bands originating from resonant multipole modes of the individual particles as well as Bragg-type modes due to the (short-range) periodicity. Strong interaction, leading to the occurrence of hybridization gaps, is observed between the acoustic band and the band of quadrupole modes of the particles that occupy the largest fractional volume of the mixed crystal; the effective radius is either that of the large (in the symmetric NaCl-type crystalline phase) or the small (in the asymmetric NaZn(13)-type crystalline phase) particles. The possibility to reveal a universal behavior of the phononic band structure for different single and binary colloidal crystalline suspensions, by representing in the dispersion diagrams reduced quantities using an appropriate length scale, is discussed.

  7. Band structures and localization properties of aperiodic layered phononic crystals

    NASA Astrophysics Data System (ADS)

    Yan, Zhi-Zhong; Zhang, Chuanzeng

    2012-03-01

    The band structures and localization properties of in-plane elastic waves with coupling of longitudinal and transverse modes oblique propagating in aperiodic phononic crystals based on Thue-Morse and Rudin-Shapiro sequences are studied. Using transfer matrix method, the concept of the localization factor is introduced and the correctness is testified through the Rytov dispersion relation. For comparison, the perfect periodic structure and the quasi-periodic Fibonacci system are also considered. In addition, the influences of the random disorder, local resonance, translational and/or mirror symmetries on the band structures of the aperiodic phononic crystals are analyzed in this paper.

  8. Phonons and defects in semiconductors and nanostructures: Phonon trapping, phonon scattering, and heat flow at heterojunctions

    SciTech Connect

    Estreicher, S. K. Gibbons, T. M.; Kang, By.; Bebek, M. B.

    2014-01-07

    Defects in semiconductors introduce vibrational modes that are distinct from bulk modes because they are spatially localized in the vicinity of the defect. Light impurities produce high-frequency modes often visible by Fourier-transform infrared absorption or Raman spectroscopy. Their vibrational lifetimes vary by orders of magnitude and sometimes exhibit unexpectedly large isotope effects. Heavy impurities introduce low-frequency modes sometimes visible as phonon replicas in photoluminescence bands. But other defects such as surfaces or interfaces exhibit spatially localized modes (SLMs) as well. All of them can trap phonons, which ultimately decay into lower-frequency bulk phonons. When heat flows through a material containing defects, phonon trapping at localized modes followed by their decay into bulk phonons is usually described in terms of phonon scattering: defects are assumed to be static scattering centers and the properties of the defect-related SLMs modes are ignored. These dynamic properties of defects are important. In this paper, we quantify the concepts of vibrational localization and phonon trapping, distinguish between normal and anomalous decay of localized excitations, discuss the meaning of phonon scattering in real space at the atomic level, and illustrate the importance of phonon trapping in the case of heat flow at Si/Ge and Si/C interfaces.

  9. Switchable topological phonon channels

    NASA Astrophysics Data System (ADS)

    Süsstrunk, Roman; Zimmermann, Philipp; Huber, Sebastian D.

    2017-01-01

    Guiding energy deliberately is one of the central elements in engineering and information processing. It is often achieved by designing specific transport channels in a suitable material. Topological metamaterials offer a way to construct stable and efficient channels of unprecedented versatility. However, due to their stability it can be tricky to terminate them or to temporarily shut them off without changing the material properties massively. While a lot of effort was put into realizing mechanical topological metamaterials, almost no works deal with manipulating their edge channels in sight of applications. Here, we take a step in this direction, by taking advantage of local symmetry breaking potentials to build a switchable topological phonon channel.

  10. Imaging carrier and phonon transport in Si using ultrashort optical pulses

    SciTech Connect

    David H. Hurley; O. B. Wright; O. Matsuda; B. E. McCandless; S. Shinde

    2009-01-01

    A series of experiments have been conducted that microscopically image thermal diffusion and surface acoustic phonon propagation within a single crystallite of a polycrystalline Si sample. The experimental approach employs ultrashort optical pulses to generate an electron-hole plasma and a second probe pulse is used to image the evolution of the plasma. By decomposing the signal into a component that varies with delay time and a steady state component that varies with pump modulation frequency, the respective influence of carrier recombination and thermal diffusion are identified. Additionally, the coherent surface acoustic phonon component to the signal is imaged using a Sagnac interferometer to monitor optical phase.

  11. Giant nonlinearity via breaking parity-time symmetry: A route to low-threshold phonon diodes

    NASA Astrophysics Data System (ADS)

    Zhang, Jing; Peng, Bo; Ã-zdemir, Şahin Kaya; Liu, Yu-xi; Jing, Hui; Lü, Xin-you; Liu, Yu-long; Yang, Lan; Nori, Franco

    2015-09-01

    Nonreciprocal devices that permit wave transmission in only one direction are indispensible in many fields of science including, e.g., electronics, optics, acoustics, and thermodynamics. Manipulating phonons using such nonreciprocal devices may have a range of applications such as phonon diodes, transistors, switches, etc. One way of achieving nonreciprocal phononic devices is to use materials with strong nonlinear response to phonons. However, it is not easy to obtain the required strong mechanical nonlinearity, especially for few-phonon situations. Here we present a general mechanism to amplify nonlinearity using parity-time (PT )-symmetric structures, and show that an on-chip microscale phonon diode can be fabricated using a PT -symmetric mechanical system, in which a lossy mechanical resonator with very weak mechanical nonlinearity is coupled to a mechanical resonator with mechanical gain but no mechanical nonlinearity. When this coupled system transits from the PT -symmetric regime to the broken-PT -symmetric regime, the mechanical nonlinearity is transferred from the lossy resonator to the one with gain, and the effective nonlinearity of the system is significantly enhanced. This enhanced mechanical nonlinearity is almost lossless because of the gain-loss balance induced by the PT -symmetric structure. Such an enhanced lossless mechanical nonlinearity is then used to control the direction of phonon propagation, and can greatly decrease (by over three orders of magnitude) the threshold of the input-field intensity necessary to observe the unidirectional phonon transport. We propose an experimentally realizable lossless low-threshold phonon diode of this type. Our study opens up perspectives for constructing on-chip few-phonon devices and hybrid phonon-photon components.

  12. Basic phononic diagnostic measurements in fluid columns

    NASA Astrophysics Data System (ADS)

    Hazony, D.; Hazony, Y.

    2010-07-01

    A pre-selected 21 MHz ultrasonic transducer was used to produce characteristic pulses, arbitrarily similar to the quantum-mechanical concept of a phonon, describable as having a single-frequency modulated Gaussian shape. The propagation of such pulses in water-acoustic channels was studied in conjunction with nonlinear regression analysis and an Erlangian model for size distribution of molecular aggregates. Experimental results obtained distinguish between surface and bulk phenomena and provide quantitative measures of an average molecular cluster size in water. The relevance of the Erlangian model, in studying the near front of the channel, provides a significant distinction between the behavior of pure water and Ringer's solution of water. The inherent consistency between the various results re-enforces the theoretical approach, implying new venues for future research.

  13. Optimal design of tunable phononic bandgap plates under equibiaxial stretch

    NASA Astrophysics Data System (ADS)

    Hedayatrasa, Saeid; Abhary, Kazem; Uddin, M. S.; Guest, James K.

    2016-05-01

    Design and application of phononic crystal (PhCr) acoustic metamaterials has been a topic with tremendous growth of interest in the last decade due to their promising capabilities to manipulate acoustic and elastodynamic waves. Phononic controllability of waves through a particular PhCr is limited only to the spectrums located within its fixed bandgap frequency. Hence the ability to tune a PhCr is desired to add functionality over its variable bandgap frequency or for switchability. Deformation induced bandgap tunability of elastomeric PhCr solids and plates with prescribed topology have been studied by other researchers. Principally the internal stress state and distorted geometry of a deformed phononic crystal plate (PhP) changes its effective stiffness and leads to deformation induced tunability of resultant modal band structure. Thus the microstructural topology of a PhP can be altered so that specific tunability features are met through prescribed deformation. In the present study novel tunable PhPs of this kind with optimized bandgap efficiency-tunability of guided waves are computationally explored and evaluated. Low loss transmission of guided waves throughout thin walled structures makes them ideal for fabrication of low loss ultrasound devices and structural health monitoring purposes. Various tunability targets are defined to enhance or degrade complete bandgaps of plate waves through macroscopic tensile deformation. Elastomeric hyperelastic material is considered which enables recoverable micromechanical deformation under tuning finite stretch. Phononic tunability through stable deformation of phononic lattice is specifically required and so any topology showing buckling instability under assumed deformation is disregarded. Nondominated sorting genetic algorithm (GA) NSGA-II is adopted for evolutionary multiobjective topology optimization of hypothesized tunable PhP with square symmetric unit-cell and relevant topologies are analyzed through finite

  14. Phonon analog of topological nodal semimetals

    NASA Astrophysics Data System (ADS)

    Po, Hoi Chun; Bahri, Yasaman; Vishwanath, Ashvin

    2016-05-01

    Topological band structures in electronic systems like topological insulators and semimetals give rise to highly unusual physical properties. Analogous topological effects have also been discussed in bosonic systems, but the novel phenomena typically occur only when the system is excited by finite-frequency probes. A mapping recently proposed by C. L. Kane and T. C. Lubensky [Nat. Phys. 10, 39 (2014), 10.1038/nphys2835], however, establishes a closer correspondence. It relates the zero-frequency excitations of mechanical systems to topological zero modes of fermions that appear at the edges of an otherwise gapped system. Here we generalize the mapping to systems with an intrinsically gapless bulk. In particular, we construct mechanical counterparts of topological semimetals. The resulting gapless bulk modes are physically distinct from the usual acoustic Goldstone phonons and appear even in the absence of continuous translation invariance. Moreover, the zero-frequency phonon modes feature adjustable momenta and are topologically protected as long as the lattice coordination is unchanged. Such protected soft modes with tunable wave vector may be useful in designing mechanical structures with fault-tolerant properties.

  15. Thermoelectric amplification of phonons in graphene

    NASA Astrophysics Data System (ADS)

    Dompreh, K. A.; Mensah, N. G.; Mensah, S. Y.; Fosuhene, S. K.

    2016-06-01

    Amplification of acoustic in-plane phonons due to an external temperature gradient (∇T) in single-layer graphene (SLG) was studied theoretically. The threshold temperature gradient (∇ T ) 0 g and the threshold voltage (V T ) 0 g in SLG were evaluated. For T = 77 K , the calculated value for (∇ T ) 0 g = 746.8 K / cm and (V T ) 0 g = 6.6 mV . The calculation was done in the hypersound regime. Further, the dependence of the normalized amplification ( Γ / Γ 0 ) on the frequency ω q and ∇ T / T were evaluated numerically and presented graphically. The calculated threshold temperature gradient (V T ) 0 g for SLG was higher than that obtained for homogeneous semiconductors (n-InSb) (∇ T ) 0 hom ≈ 10 3 K / cm , superlattices (∇ T ) 0 S L ≈ 384 K / cm , and cylindrical quantum wire (∇ T ) 0 c q w ≈ 10 2 K / cm . This makes SLG a much better material for thermoelectric phonon amplification.

  16. An Artificial Ising System with Phononic Excitations

    NASA Astrophysics Data System (ADS)

    Ghaffari, Hamed; Griffith, W. Ashley; Benson, Philip; Nasseri, M. H. B.; Young, R. Paul

    Many intractable systems and problems can be reduced to a system of interacting spins. Here, we report mapping collective phononic excitations from different sources of crystal vibrations to spin systems. The phononic excitations in our experiments are due to micro and nano cracking (yielding crackling noises due to lattice distortion). We develop real time mapping of the multi-array senores to a network-space and then mapping the excitation- networks to spin-like systems. We show that new mapped system satisfies the quench (impulsive) characteristics of the Ising model in 2D classical spin systems. In particular, we show that our artificial Ising system transits between two ground states and approaching the critical point accompanies with a very short time frozen regime, inducing formation of domains separated by kinks. For a cubic-test under a true triaxial test (3D case), we map the system to a 6-spin ring under a transversal-driving field where using functional multiplex networks, the vector components of the spin are inferred (i.e., XY model). By visualization of spin patterns of the ring per each event, we demonstrate that ``kinks'' (as defects) proliferate when system approach from above to its critical point. We support our observations with employing recorded acoustic excitations during distortion of crystal lattices in nano-indentation tests on different crystals (silicon and graphite), triaxial loading test on rock (poly-crystal) samples and a true 3D triaxial test.

  17. Raman electron spin-lattice relaxation with the Debye-type and with real phonon spectra in crystals

    NASA Astrophysics Data System (ADS)

    Hoffmann, Stanislaw K.; Lijewski, Stefan

    2013-02-01

    Electron spin-lattice relaxation temperature dependence was measured for Ti2+ (S = 1) and for Cu2+ (S = 1/2) ions in SrF2 single crystal by electron spin echo method in temperature range 4-109 K. The spin relaxation was governed by the two-phonon Raman processes. The relaxation theory is outlined and presented in a form suitable for applying with real phonon spectra. The experimental relaxation results were described using Debye-type phonon spectrum and the real phonon spectrum of SrF2 crystal. The Debye approximation does not fit well the results for SrF2 both at low and at high temperature. The relaxation rate is faster than that predicted by Debye-type phonon spectrum at low temperatures where excess of lattice vibrations over the Debye model exists but is slower at higher temperatures (above 50 K) where density of phonon states continuously decreases when approaching to the maximal acoustic phonon frequency. The expected deviation from Debye approximation was analyzed also for Cu2+ in NaCl and MgSiO3 crystals for which phonon spectra are available. The fitting with the real phonon spectrum allowed us to calculate spin-phonon coupling parameter as 267 cm-1 for Ti2+ and 1285 cm-1 for Cu2+ in SrF2.

  18. Two-Phonon Absorption

    ERIC Educational Resources Information Center

    Hamilton, M. W.

    2007-01-01

    A nonlinear aspect of the acousto-optic interaction that is analogous to multi-photon absorption is discussed. An experiment is described in which the second-order acousto-optically scattered intensity is measured and found to scale with the square of the acoustic intensity. This experiment using a commercially available acousto-optic modulator is…

  19. Electron-phonon coupling and thermal transport in the thermoelectric compound Mo3Sb7–xTex

    DOE PAGES

    Bansal, Dipanshu; Li, Chen W.; Said, Ayman H.; ...

    2015-12-07

    Phonon properties of Mo3Sb7–xTex (x = 0, 1.5, 1.7), a potential high-temperature thermoelectric material, have been studied with inelastic neutron and x-ray scattering, and with first-principles simulations. The substitution of Te for Sb leads to pronounced changes in the electronic struc- ture, local bonding, phonon density of states (DOS), dispersions, and phonon lifetimes. Alloying with tellurium shifts the Fermi level upward, near the top of the valence band, resulting in a strong suppression of electron-phonon screening, and a large overall stiffening of interatomic force- constants. The suppression in electron-phonon coupling concomitantly increases group velocities and suppresses phonon scattering rates, surpassingmore » the effects of alloy-disorder scattering, and re- sulting in a surprising increased lattice thermal conductivity in the alloy. We also identify that the local bonding environment changes non-uniformly around different atoms, leading to variable perturbation strengths for different optical phonon branches. The respective roles of changes in phonon group velocities and phonon lifetimes on the lattice thermal conductivity are quantified. Lastly, our results highlight the importance of the electron-phonon coupling on phonon mean-free-paths in this compound, and also estimates the contributions from boundary scattering, umklapp scattering, and point-defect scattering.« less

  20. Electron-phonon coupling and thermal conductance at a metal-semiconductor interface: First-principles analysis

    SciTech Connect

    Sadasivam, Sridhar; Fisher, Timothy S.; Waghmare, Umesh V.

    2015-04-07

    The mechanism of heat transfer and the contribution of electron-phonon coupling to thermal conductance of a metal-semiconductor interface remains unclear in the present literature. We report ab initio simulations of a technologically important titanium silicide (metal)–silicon (semiconductor) interface to estimate the Schottky barrier height, and the strength of electron-phonon and phonon-phonon heat transfer across the interface. The electron and phonon dispersion relations of TiSi{sub 2} with C49 structure and the TiSi{sub 2}-Si interface are obtained using first-principles calculations within the density functional theory framework. These are used to estimate electron-phonon linewidths and the associated Eliashberg function that quantifies coupling. We show that the coupling strength of electrons with interfacial phonon modes is of the same order of magnitude as coupling of electrons to phonon modes in the bulk metal, and its contribution to electron-phonon interfacial conductance is comparable to the harmonic phonon-phonon conductance across the interface.

  1. Structural engineering of three-dimensional phononic crystals

    NASA Astrophysics Data System (ADS)

    Delpero, Tommaso; Schoenwald, Stefan; Zemp, Armin; Bergamini, Andrea

    2016-02-01

    Artificially-structured materials are attracting the research interest of a growing community of scientists for the possibility to develop novel materials with advantageous properties that arise from the ability to tailor the propagation of elastic waves, and thus energy, through them. In this work, we propose a three-dimensional phononic crystal whose unit cell has been engineered to obtain a strong wave-attenuation band in the middle of the acoustic frequency range. The combination of its acoustic properties with the dimensions of the unit cell and its static mechanical properties makes it an interesting material for possibly several applications in civil and mechanical engineering, for instance as the core of an acoustically insulating sandwich panel. A sample of this crystal has been manufactured and experimentally tested with respect to its acoustic transmissibility. The performance of the phononic crystal core is remarkable both in terms of amplitude reduction in the transmissibility and width of the attenuation band. A parametric study has been finally conducted on selected geometrical parameters of the unit cell and on their effect on the macroscopic properties of the crystal. This work represents an application-oriented example of how the macroscopic properties of an artificially-structured material can be designed, according to specific needs, by a conventional engineering of its unit cell.

  2. Topological phononic states of underwater sound based on coupled ring resonators

    SciTech Connect

    He, Cheng; Li, Zheng; Ni, Xu; Sun, Xiao-Chen; Yu, Si-Yuan; Lu, Ming-Hui Liu, Xiao-Ping; Chen, Yan-Feng

    2016-01-18

    We report a design of topological phononic states for underwater sound using arrays of acoustic coupled ring resonators. In each individual ring resonator, two degenerate acoustic modes, corresponding to clockwise and counter-clockwise propagation, are treated as opposite pseudospins. The gapless edge states arise in the bandgap resulting in protected pseudospin-dependent sound transportation, which is a phononic analogue of the quantum spin Hall effect. We also investigate the robustness of the topological sound state, suggesting that the observed pseudospin-dependent sound transportation remains unless the introduced defects facilitate coupling between the clockwise and counter-clockwise modes (in other words, the original mode degeneracy is broken). The topological engineering of sound transportation will certainly promise unique design for next generation of acoustic devices in sound guiding and switching, especially for underwater acoustic devices.

  3. Multi-band asymmetric acoustic transmission in a bended waveguide with multiple mechanisms

    NASA Astrophysics Data System (ADS)

    Huang, Yu-lei; Sun, Hong-xiang; Xia, Jian-ping; Yuan, Shou-qi; Ding, Xin-lei

    2016-07-01

    We report the realization of a multi-band device of the asymmetric acoustic transmission by placing a phononic crystal inside a bended waveguide immersed in water, as determined both experimentally and numerically. The asymmetric acoustic transmission exists in three frequency bands below 500 kHz induced by multiple mechanisms. Besides the band gap of the phononic crystal, we also introduce the deaf mode and interaction between the phononic crystal and waveguide. More importantly, this asymmetric transmission can be systematically controlled by mechanically rotating the square rods of the phononic crystal. The device has the advantages of multiple band, broader bandwidth, and adjustable property, showing promising applications in ultrasonic devices.

  4. Phonon transport analysis of semiconductor nanocomposites using monte carlo simulations

    NASA Astrophysics Data System (ADS)

    Malladi, Mayank

    computed by using both gray media and non-gray media approaches. The non-gray media simulations take into consideration the dispersion and polarization effects of phonon transport. The effects of volume fraction, size, shape and distribution of the nanowire fillers on heat flow and hence thermal conductivity are studied. In addition, the computational performances of the gray and non-gray media approaches are compared.

  5. First-principles investigations of phonon anharmonicity and electronic instability in thermoelectric SnSe

    NASA Astrophysics Data System (ADS)

    Hong, Jiawang; Li, Chen W.; May, A. F.; Bansal, D.; Chi, S.; Hong, T.; Ehlers, G.; Delaire, Olivier

    The promising thermoelectric material SnSe exhibits ultra-low and strongly anisotropic thermal conductivity. By combining first-principles calculations and inelastic neutron scattering measurements, we have investigated the phonon dispersions and phonon scattering mechanisms, and probed the origin of the large anharmonicity in SnSe. We will discuss the connection between the phonon properties and the high-temperature structural phase transition, and how the electronic structure leads to large anharmonic phonon interactions in SnSe. The present results provide a microscopic picture connecting electronic structure and phonon anharmonicity in SnSe, which could help design materials with ultralow thermal conductivity. Computations were performed using the OLCF at ORNL. Modeling of neutron data was performed in CAMM, measurements were funded by the US DOE, BES, Materials Science and Engineering Division.

  6. A study of phonon anisotropic scattering effect on silicon thermal conductivity at nanoscale

    SciTech Connect

    Bong, Victor N-S; Wong, Basil T.

    2015-08-28

    Previous studies have shown that anisotropy in phonon transport exist because of the difference in phonon dispersion relation due to different lattice direction, as observed by a difference in in-plane and cross-plane thermal conductivity. The directional preference (such as forward or backward scattering) in phonon propagation however, remains a relatively unexplored frontier. Our current work adopts a simple scattering probability in radiative transfer, which is called Henyey and Greenstein probability density function, and incorporates it into the phonon Monte Carlo simulation to investigate the effect of directional scattering in phonon transport. In this work, the effect of applying the anisotropy scattering is discussed, as well as its impact on the simulated thermal conductivity of silicon thin films. While the forward and backward scattering will increase and decrease thermal conductivity respectively, the extent of the effect is non-linear such that forward scattering has a more obvious effect than backward scattering.

  7. Dynamics of a vertical cavity quantum cascade phonon laser structure

    NASA Astrophysics Data System (ADS)

    Maryam, W.; Akimov, A. V.; Campion, R. P.; Kent, A. J.

    2013-07-01

    Driven primarily by scientific curiosity, but also by the potential applications of intense sources of coherent sound, researchers have targeted the phonon laser (saser) since the invention of the optical laser over 50 years ago. Here we fabricate a vertical cavity structure designed to operate as a saser oscillator device at a frequency of 325 GHz. It is based on a semiconductor superlattice gain medium, inside a multimode cavity between two acoustic Bragg reflectors. We measure the acoustic output of the device as a function of time after applying electrical pumping. The emission builds in intensity reaching a steady state on a timescale of order 0.1 μs. We show that the results are consistent with a model of the dynamics of a saser cavity exactly analogous to the models used for describing laser dynamics. We also obtain estimates for the gain coefficient, steady-state acoustic power output and efficiency of the device.

  8. THz Acoustic Spectroscopy by using Double Quantum Wells and Ultrafast Optical Spectroscopy

    PubMed Central

    Wei, Fan Jun; Yeh, Yu-Hsiang; Sheu, Jinn-Kong; Lin, Kung-Hsuan

    2016-01-01

    GaN is a pivotal material for acoustic transducers and acoustic spectroscopy in the THz regime, but its THz phonon properties have not been experimentally and comprehensively studied. In this report, we demonstrate how to use double quantum wells as a THz acoustic transducer for measuring generated acoustic phonons and deriving a broadband acoustic spectrum with continuous frequencies. We experimentally investigated the sub-THz frequency dependence of acoustic attenuation (i.e., phonon mean-free paths) in GaN, in addition to its physical origins such as anharmonic scattering, defect scattering, and boundary scattering. A new upper limit of attenuation caused by anharmonic scattering, which is lower than previously reported values, was obtained. Our results should be noteworthy for THz acoustic spectroscopy and for gaining a fundamental understanding of heat conduction. PMID:27346494

  9. Confinement of phonon propagation in laser deposited tungsten/polycarbonate multilayers

    NASA Astrophysics Data System (ADS)

    Döring, Florian; Ulrichs, Henning; Pagel, Sinja; Müller, Markus; Mansurova, Maria; Müller, Matthias; Eberl, Christian; Erichsen, Torben; Huebner, Dennis; Vana, Philipp; Mann, Klaus; Münzenberg, Markus; Krebs, Hans-Ulrich

    2016-09-01

    Nanoscale multilayer thin films of W and PC (Polycarbonate) show, due to the great difference of the components’ characteristics, fascinating properties for a variety of possible applications and provide an interesting research field, but are hard to fabricate with low layer thicknesses. Because of the great acoustic mismatch between the two materials, such nanoscale structures are promising candidates for new phononic materials, where phonon propagation is strongly reduced. In this article we show for the first time that W/PC-multilayers can indeed be grown with high quality by pulsed laser deposition. We analyzed the polymer properties depending on the laser fluence used for deposition, which enabled us to find best experimental conditions for the fabrication of high-acoustic-mismatch W/PC multilayers. The multilayers were analyzed by fs pump-probe spectroscopy showing that phonon dynamics on the ps time-scale can strongly be tailored by structural design. While already periodic multilayers exhibit strong phonon localization, especially aperiodic structures present outstandingly low phonon propagation properties making such 1D-layered W/PC nano-structures interesting for new phononic applications.

  10. Phonon spectra of alkali metals

    NASA Astrophysics Data System (ADS)

    Zeković, S.; Vukajlović, F.; Veljković, V.

    1982-10-01

    In this work we used a simple local model pseudopotential which includes screening for the phonon spectra calculations of alkali metals. The results obtained are in very good agreement with experimental data. In some branches of phonon spectra the differences between theoretical and experimental results are within 1-2%, while the maximum error is about 6%. The suggested form of the pseudopotential allows us to describe the phonon spectra of Na, K and Rb with only one, and, at the same time, a unique, parameter. In this case, the maximum disagreements from experiment are 9% for Na, 8% for K and 7% for Rb.

  11. Electron-Phonon Coupling and Energy Flow in a Simple Metal beyond the Two-Temperature Approximation

    NASA Astrophysics Data System (ADS)

    Waldecker, Lutz; Bertoni, Roman; Ernstorfer, Ralph; Vorberger, Jan

    2016-04-01

    The electron-phonon coupling and the corresponding energy exchange are investigated experimentally and by ab initio theory in nonequilibrium states of the free-electron metal aluminium. The temporal evolution of the atomic mean-squared displacement in laser-excited thin freestanding films is monitored by femtosecond electron diffraction. The electron-phonon coupling strength is obtained for a range of electronic and lattice temperatures from density functional theory molecular dynamics simulations. The electron-phonon coupling parameter extracted from the experimental data in the framework of a two-temperature model (TTM) deviates significantly from the ab initio values. We introduce a nonthermal lattice model (NLM) for describing nonthermal phonon distributions as a sum of thermal distributions of the three phonon branches. The contributions of individual phonon branches to the electron-phonon coupling are considered independently and found to be dominated by longitudinal acoustic phonons. Using all material parameters from first-principles calculations except the phonon-phonon coupling strength, the prediction of the energy transfer from electrons to phonons by the NLM is in excellent agreement with time-resolved diffraction data. Our results suggest that the TTM is insufficient for describing the microscopic energy flow even for simple metals like aluminium and that the determination of the electron-phonon coupling constant from time-resolved experiments by means of the TTM leads to incorrect values. In contrast, the NLM describing transient phonon populations by three parameters appears to be a sufficient model for quantitatively describing electron-lattice equilibration in aluminium. We discuss the general applicability of the NLM and provide a criterion for the suitability of the two-temperature approximation for other metals.

  12. Engineering absorption and blackbody radiation in the far-infrared with surface phonon polaritons on gallium phosphide

    SciTech Connect

    Streyer, W.; Law, S.; Rosenberg, A.; Wasserman, D.; Roberts, C.; Podolskiy, V. A.; Hoffman, A. J.

    2014-03-31

    We demonstrate excitation of surface phonon polaritons on patterned gallium phosphide surfaces. Control over the light-polariton coupling frequencies is demonstrated by changing the pattern periodicity and used to experimentally determine the gallium phosphide surface phonon polariton dispersion curve. Selective emission via out-coupling of thermally excited surface phonon polaritons is experimentally demonstrated. Samples are characterized experimentally by Fourier transform infrared reflection and emission spectroscopy, and modeled using finite element techniques and rigorous coupled wave analysis. The use of phonon resonances for control of emissivity and excitation of bound surface waves offers a potential tool for the exploration of long-wavelength Reststrahlen band frequencies.

  13. Low-energy phonons and superconductivity in Sn0.8In0.2Te

    NASA Astrophysics Data System (ADS)

    Xu, Zhijun; Schneeloch, J. A.; Zhong, R. D.; Rodriguez-Rivera, J. A.; Harriger, L. W.; Birgeneau, R. J.; Gu, G. D.; Tranquada, J. M.; Xu, Guangyong

    2015-02-01

    We present neutron scattering measurements on low-energy phonons from a superconducting (Tc=2.7 K ) Sn0.8In0.2Te single-crystal sample. The longitudinal acoustic phonon mode and one transverse acoustic branch have been mapped out around the (002) Bragg peak for temperatures of 1.7 and 4.2 K. We observe a substantial energy width of the transverse phonons at energies comparable to twice the superconducting gap; however, there is no change in this width between the superconducting and normal states, and the precise origin of this energy width anomaly is not entirely clear. We also confirm that the compound is well ordered, with no indications of structural instability.

  14. YPHON: A package for calculating phonons of polar materials

    NASA Astrophysics Data System (ADS)

    Wang, Yi; Chen, Long-Qing; Liu, Zi-Kui

    2014-11-01

    In our recent works, we have developed a mixed-space approach within the framework of direct method for the first-principle calculation of phonon properties. It makes full use of the accuracy of the force constants calculated in the real space and the dipole-dipole interactions in the reciprocal space, making the accurate phonon calculation possible with the direct method for polar materials. In this paper, an efficient C++ implementation of the mixed-space approach, YPHON, is provided as open source, including demos and Linux scripts for extracting input data to YPHON from the output of VASP.5. The functions of the current package include the calculations of: (1) the phonon dispersions; (2) the phonon density of states; (3) the neutron scattering section weighted phonon density of state; (4) the phonons of the high symmetry structure using the force constants from low symmetry structure; (5) the phonon dispersions of random alloys; and (6) the analysis of the vibrational modes using the point group theory. Catalogue identifier: AETS_v1_0 Program summary URL:http://cpc.cs.qub.ac.uk/summaries/AETS_v1_0.html Program obtainable from: CPC Program Library, Queen’s University, Belfast, N. Ireland Licensing provisions: Standard CPC licence, http://cpc.cs.qub.ac.uk/licence/licence.html No. of lines in distributed program, including test data, etc.: 567815 No. of bytes in distributed program, including test data, etc.: 9763594 Distribution format: tar.gz Programming language: C++, Linux scripts. Computer: Linux systems with a g++ or C++ compiler. Operating system: Linux. RAM: Ranges from a few Mbytes to a few Gbytes, dynamically depending on the system size. Classification: 7.8. External routines: GSL-the GNU Scientific Library (GSL) is a numerical library for C and C++ programmers. VASP.5 or later for the calculations of force constants and dielectric constants and Born effective charge for polar materials. Nature of problem: This package has the purpose of computing

  15. Acoustic studies of solids

    SciTech Connect

    Granato, A.V.

    1987-01-01

    Acoustic technique have proven to be very useful in getting basic information on the configuration and dynamics of defects. Although the technique is indirect, the sensitivity is such that it often competes very favorably with more direct techniques such as neutron, x-ray, or phonon scattering. The symmetry information that comes directly from polarization control often also proves decisive in determining configurations. Many of the concepts that have been developed in explaining the various effects that have been seen in dislocation and point defect studies have proven also to be very useful when taken over almost directly into other areas of physics. 11 refs., 7 figs.

  16. Low-temperature semiconductor band-gap thermal shifts: T4 shifts from ordinary acoustic and T2 from piezoacoustic coupling

    NASA Astrophysics Data System (ADS)

    Allen, Philip B.; Nery, Jean Paul

    2017-01-01

    At low temperature, the experimental gap of silicon decreases as Eg(T ) =Eg(0 ) -A T4 . The main reason is electron-phonon renormalization. The physics behind the T4-power law is more complex than has been realized. Renormalization at low T by intraband scattering requires a nonadiabatic treatment in order to correctly include acoustic phonons and avoid divergences from piezoacoustic phonon interactions. The result is an unexpected low T term Eg(0 ) +A'Tp with positive coefficient A', and power p =4 for nonpiezoelectric materials, and power p =2 for piezoelectric materials. The acoustic phonons in piezoelectric semiconductors generate a piezoelectric field, modifying the electron-phonon coupling. However, at higher T , thermally excited acoustic phonons of energy ℏ vsq and intraband excitation energies ɛq-ɛ0=ℏ2q2/2 m* become comparable in size. Above this temperature, the low q and higher q intraband acoustic phonon contributions to Tp rapidly cancel, leaving little thermal effect. Then the contribution from interband scattering by acoustic phonons is dominant. This has the power law T4 for both nonpiezoelectric and piezoelectric semiconductors. The shift can then have either sign, but usually reduces the size of gaps as T increases. It arises after cancellation of the T2 terms that appear separately in Debye-Waller and Fan parts of the acoustic phonon interband renormalization. The cancellation occurs because of the acoustic sum rule.

  17. 25th Anniversary Article: Ordered Polymer Structures for the Engineering of Photons and Phonons

    PubMed Central

    Lee, Jae-Hwang; Koh, Cheong Yang; Singer, Jonathan P; Jeon, Seog-Jin; Maldovan, Martin; Stein, Ori; Thomas, Edwin L

    2014-01-01

    The engineering of optical and acoustic material functionalities via construction of ordered local and global architectures on various length scales commensurate with and well below the characteristic length scales of photons and phonons in the material is an indispensable and powerful means to develop novel materials. In the current mature status of photonics, polymers hold a pivotal role in various application areas such as light-emission, sensing, energy, and displays, with exclusive advantages despite their relatively low dielectric constants. Moreover, in the nascent field of phononics, polymers are expected to be a superior material platform due to the ability for readily fabricated complex polymer structures possessing a wide range of mechanical behaviors, complete phononic bandgaps, and resonant architectures. In this review, polymer-centric photonic and phononic crystals and metamaterials are highlighted, and basic concepts, fabrication techniques, selected functional polymers, applications, and emerging ideas are introduced. PMID:24338738

  18. 25th anniversary article: ordered polymer structures for the engineering of photons and phonons.

    PubMed

    Lee, Jae-Hwang; Koh, Cheong Yang; Singer, Jonathan P; Jeon, Seog-Jin; Maldovan, Martin; Stein, Ori; Thomas, Edwin L

    2014-01-01

    The engineering of optical and acoustic material functionalities via construction of ordered local and global architectures on various length scales commensurate with and well below the characteristic length scales of photons and phonons in the material is an indispensable and powerful means to develop novel materials. In the current mature status of photonics, polymers hold a pivotal role in various application areas such as light-emission, sensing, energy, and displays, with exclusive advantages despite their relatively low dielectric constants. Moreover, in the nascent field of phononics, polymers are expected to be a superior material platform due to the ability for readily fabricated complex polymer structures possessing a wide range of mechanical behaviors, complete phononic bandgaps, and resonant architectures. In this review, polymer-centric photonic and phononic crystals and metamaterials are highlighted, and basic concepts, fabrication techniques, selected functional polymers, applications, and emerging ideas are introduced.

  19. Phonon symmetries in hexagonal boron nitride probed by incoherent light emission

    NASA Astrophysics Data System (ADS)

    Vuong, T. Q. P.; Cassabois, G.; Valvin, P.; Jacques, V.; Van Der Lee, A.; Zobelli, A.; Watanabe, K.; Taniguchi, T.; Gil, B.

    2017-03-01

    Layered compounds are stacks of weakly bound two-dimensional atomic crystals, with a prototypal hexagonal structure in graphene, transition metal dichalcogenides and boron nitride. This crystalline anisotropy results in vibrational modes with specific symmetries depending on the in-plane or out-of-plane atomic displacements. We show that polarization-resolved photoluminescence measurements in hexagonal boron nitride reflect the phonon symmetries in this layered semiconductor. Experiments performed with a detection on the sample edge, perpendicular to the c-axis, reveal the strong polarization-dependence of the emission lines corresponding to the recombination assisted by the three acoustic phonon modes. We elucidate the dipole orientation of the fundamental indirect exciton. We demonstrate evidence of the so-far missing phonon replica due to the optical out-of-plane phonon mode.

  20. Band structures of two dimensional solid/air hierarchical phononic crystals

    NASA Astrophysics Data System (ADS)

    Xu, Y. L.; Tian, X. G.; Chen, C. Q.

    2012-06-01

    The hierarchical phononic crystals to be considered show a two-order “hierarchical” feature, which consists of square array arranged macroscopic periodic unit cells with each unit cell itself including four sub-units. Propagation of acoustic wave in such two dimensional solid/air phononic crystals is investigated by the finite element method (FEM) with the Bloch theory. Their band structure, wave filtering property, and the physical mechanism responsible for the broadened band gap are explored. The corresponding ordinary phononic crystal without hierarchical feature is used for comparison. Obtained results show that the solid/air hierarchical phononic crystals possess tunable outstanding band gap features, which are favorable for applications such as sound insulation and vibration attenuation.

  1. Coupling of nitrogen vacancy centres in nanodiamonds by means of phonons

    NASA Astrophysics Data System (ADS)

    Albrecht, A.; Retzker, A.; Jelezko, F.; Plenio, M. B.

    2013-08-01

    Realizing controlled quantum dynamics via the magnetic interactions between colour centres in diamond remains a challenge despite recent demonstrations for nanometre separated pairs. Here we propose to use the intrinsic acoustical phonons in diamond as a data bus for accomplishing this task. We show that for nanodiamonds the electron-phonon coupling can take significant values that together with mode frequencies in the THz range can serve as a resource for conditional gate operations. Based on these results, we analyse how to use this phonon-induced interaction for constructing quantum gates among the electron-spin triplet ground states, introducing the phonon dependence via Raman transitions. Combined with decoupling pulses this offers the possibility for creating entangled states within nanodiamonds on the scale of several tens of nanometres, a promising prerequisite for quantum sensing applications.

  2. Investigation of locally resonant absorption and factors affecting the absorption band of a phononic glass

    NASA Astrophysics Data System (ADS)

    Chen, Meng; Jiang, Heng; Feng, Yafei; Wang, Yuren

    2014-12-01

    We experimentally and theoretically investigated the mechanisms of acoustic absorption in phononic glass to optimize its properties. First, we experimentally studied its locally resonant absorption mechanism. From these results, we attributed its strong sound attenuation to its locally resonant units and its broadband absorption to its networked structure. These experiments also indicated that the porosity and thickness of the phononic glass must be tuned to achieve the best sound absorption at given frequencies. Then, using lumped-mass methods, we studied how the absorption bandgaps of the phononic glass were affected by various factors, including the porosity and the properties of the coating materials. These calculations gave optimal ranges for selecting the porosity, modulus of the coating material, and ratio of the compliant coating to the stiff matrix to achieve absorption bandgaps in the range of 6-30 kHz. This paper provides guidelines for designing phononic glasses with proper structures and component materials to work in specific frequency ranges.

  3. Phonon dynamics of neptunium chalcogenides

    NASA Astrophysics Data System (ADS)

    Aynyas, Mahendra; Rukmangad, Aditi; Arya, Balwant S.; Sanyal, Sankar P.

    2012-06-01

    We have performed phonon calculations of Neptunium Chalcogenides (NpX) (X= S, Se, Te) based on breathing shell model (BSM) which includes breathing motion of electron of the Np-atoms due to f-d hybridization. The model predicts that the short range breathing phenomenon play a dominant role in the phonon properties. We also report, for the first time specific heat for these compounds.

  4. Evidence of a Love wave bandgap in a quartz substrate coated with a phononic thin layer

    SciTech Connect

    Liu, Ting-Wei; Wu, Tsung-Tsong; Lin, Yu-Ching; Tsai, Yao-Chuan; Ono, Takahito; Tanaka, Shuji

    2014-05-05

    This paper presents a numerical and experimental study of Love wave propagation in a micro-fabricated phononic crystal (PC) structure consisting of a 2D, periodically etched silica film deposited on a quartz substrate. The dispersion characteristics of Love waves in such a phononic structure were analyzed with various geometric parameters by using complex band structure calculations. For the experiment, we adopted reactive-ion etching with electron-beam lithography to fabricate a submicrometer phononic structure. The measured results exhibited consistency with the numerical prediction. The results of this study may serve as a basis for developing PC-based Love wave devices.

  5. Phonons and phase stability in Ti-V approximants to gum metal

    NASA Astrophysics Data System (ADS)

    Hanlumyuang, Y.; Sankaran, R. P.; Sherburne, M. P.; Morris, J. W., Jr.; Chrzan, D. C.

    2012-04-01

    The stability of competing phases within body-centered-cubic Ti-V approximants to gum metal is considered from the perspective of phonon dispersion. Phonons are associated with the potential to form the ω and α'' phases. It is argued that alloys can be designed to be linearly stable with respect to the formation of both phases, even as the ideal shear strength approaches zero. The reduction in ideal strength is associated with softening of the phonons along Γ-N and is reflected in diffuse-scattering diffraction experiments.

  6. Phonons in the ordered c(2 × 2) phases of Na and Li on Al(001).

    PubMed

    Rusina, G G; Eremeev, S V; Borisova, S D; Sklyadneva, I Yu; Echenique, P M; Chulkov, E V

    2007-07-04

    The vibrational properties of the Al(001)-c(2 × 2)-Na (Li) ordered phases formed by alkali atoms (Na and Li) on the Al(001) surface at low and room temperatures are presented. The equilibrium structural characteristics, phonon dispersions and polarization of vibrational modes as well as the local density of phonon states are calculated using the embedded-atom method. The obtained structural parameters are in close agreement with experimental data.

  7. Phonons in the ordered c(2 × 2) phases of Na and Li on Al(001)

    NASA Astrophysics Data System (ADS)

    Rusina, G. G.; Eremeev, S. V.; Borisova, S. D.; Sklyadneva, I. Yu; Echenique, P. M.; Chulkov, E. V.

    2007-07-01

    The vibrational properties of the Al(001)-c(2 × 2)-Na (Li) ordered phases formed by alkali atoms (Na and Li) on the Al(001) surface at low and room temperatures are presented. The equilibrium structural characteristics, phonon dispersions and polarization of vibrational modes as well as the local density of phonon states are calculated using the embedded-atom method. The obtained structural parameters are in close agreement with experimental data.

  8. Electron and Phonon Dynamics in Hexagonal Pd Nanosheets and Ag/Pd/Ag Sandwich Nanoplates.

    PubMed

    Wang, Li; Sagaguchi, Takuya; Okuhata, Tomoki; Tsuboi, Motohiro; Tamai, Naoto

    2017-02-28

    Pd and its hybrid nanostructures have attracted considerable attention over the past decade, with both catalytic and plasmonic properties. The electron and phonon properties directly govern conversion efficiencies in applications such as energy collectors and photocatalysts. We report the dynamic processes of electron-phonon coupling and coherent acoustic phonon vibration in hexagonal Pd nanosheets and Ag/Pd/Ag sandwich nanoplates using transient absorption spectroscopy. The electron-phonon coupling constant of Pd nanosheets, GPd-nanosheet (8.7 × 10(17) W/(m(3)·K)) is larger than that of the bulk GPd (5.0 × 10(17) W/(m(3)·K)). The effective coupling constant Geff of Ag/Pd/Ag nanoplates decreases with increasing Ag shell thickness, finally approaching the bulk GAg. The variation of Geff is explained in terms of reduced density of states near Fermi level of Pd nanosheets with 1.8 nm ultrathin thickness. Coherent acoustic phonon vibration in Pd nanosheets is assigned to a fundamental breathing mode, similar to the vibration of benzene. The period increases with increasing Ag shell thickness. For Ag/Pd/Ag nanoplates with 20 nm thick Ag shells, the vibrational mode is ascribed to a quasi-extensional mode. The results show that the modes of the coherent acoustic phonon vibration transform with the geometric variation of Pd nanosheets and Ag/Pd/Ag nanoplates. Our results represent an understanding of quantum-confinement related electron dynamics and bulk-like phonon kinetics in the ultrathin Pd nanosheets and their hybrid nanostructures.

  9. Femtosecond time-resolved study of the generation and propagation of phonon polaritons in LiNbO3

    NASA Astrophysics Data System (ADS)

    Planken, P. C. M.; Noordam, L. D.; Kennis, J. T. M.; Lagendijk, A.

    1992-04-01

    Using intense femtosecond pulses, we have generated phonon polaritons in the ferroelectric crystal LiNbO3. Phonon-polariton pulses consisting of ~=8 oscillations of the electric field were generated. They were detected in a time-resolved way by diffraction of a probe pulse from the standing wave formed by these phonon polaritons. We determined their dispersion for frequencies up to 130 cm-1. The pulse width of the phonon polaritons was ~=3 ps. In addition, we have studied their propagation in the crystal, by diffracting a probe pulse from one of the traveling phonon polaritons. We demonstrate that in this case, the diffracted signal is sensitive to the phase of the phonon polariton. Analytical calculations show that this can be explained in terms of the interference between the electric fields of the nondiffracted probe beam and the first-order diffracted probe beam.

  10. Phonon scattering due to van der Waals forces in the lattice thermal conductivity of Bi2Te3 thin films

    NASA Astrophysics Data System (ADS)

    Park, Kyeong Hyun; Mohamed, Mohamed; Aksamija, Zlatan; Ravaioli, Umberto

    2015-01-01

    In this work, we calculate the thermal conductivity of layered bismuth telluride (Bi2Te3) thin films by solving the Boltzmann transport equation in the relaxation-time approximation using full phonon dispersion and compare our results with recently published experimental data and molecular dynamics simulation. The group velocity of each phonon mode is readily extracted from the full phonon dispersion obtained from first-principle density-functional theory calculation and is used along with the phonon frequency to compute the various scattering terms. Our model incorporates the typical interactions impeding thermal transport (e.g., umklapp, isotope, and boundary scatterings) and introduces a new interaction capturing the reduction of phonon transmission through van der Waals interfaces of adjacent Bi2Te3 quintuple layers forming the virtual superlattice thin film. We find that this novel approach extends the empirical Klemens-Callaway relaxation model in such anisotropic materials and recovers the experimental anisotropy while using a minimal set of parameters.

  11. Giant Anharmonic Phonon Scattering in PbTe

    SciTech Connect

    Delaire, Olivier A; Ma, Jie; Marty, Karol J; May, Andrew F; McGuire, Michael A; Singh, David J; Lumsden, Mark D; Sales, Brian C; Du, Mao-Hua; Ehlers, Georg; Podlesnyak, Andrey A

    2011-01-01

    Understanding the microscopic processes affecting the bulk thermal conductivity is crucial to develop more efficient thermoelectric materials. PbTe is currently one of the leading thermoelectric materials, largely thanks to its low thermal conductivity. However, the origin of this low thermal conductivity in a simple rocksalt structure has so far been elusive. Using a combination of inelastic neutron scattering measurements and first-principles computations of the phonons, we identify a strong anharmonic coupling between the ferroelectric transverse optic (TO) mode and the longitudinal acoustic (LA) modes in PbTe. This interaction extends over a large portion of reciprocal space, and directly affects the heat-carrying LA phonons. The LA-TO anharmonic coupling is likely to play a central role in explaining the low thermal conductivity of PbTe. The present results provide a microscopic picture of why many good thermoelectric materials are found near a lattice instability of the ferroelectric type.

  12. Anomalous phonon characteristics of unconventional novel III-N superlattices

    SciTech Connect

    Talwar, Devki N.

    2014-03-31

    Comprehensive results of atomic vibrations are reported in the unconventional short-period zb BN/GaN superlatices (SLs) by exploiting a rigid-ion-model and taking into account both the short- and long-range Coulomb interactions. Besides anisotropic mode behavior of optical phonons, our study provided evidence of acoustic-mode anti-crossing, mini-gap formation, confinement as well as BN-like modes falling within the gap that separates optical phonon bands of the two materials. A bond-polarizability scheme is employed within the second-nearest-neighbor linear-chain model to simulate the Raman intensity profiles of BN/GaN SLs revealing major expected trends of the vibrational characteristics observed experimentally in many conventional superlattice systems while eliciting some interesting contrasts.

  13. Nontrivial contribution of Fröhlich electron-phonon interaction to lattice thermal conductivity of wurtzite GaN

    NASA Astrophysics Data System (ADS)

    Yang, Jia-Yue; Qin, Guangzhao; Hu, Ming

    2016-12-01

    The macroscopic thermal transport is fundamentally determined by the intrinsic interactions among microscopic electrons and phonons. In conventional insulators and semiconductors, phonons dominate the thermal transport, and the contribution of electron-phonon interaction (EPI) is negligible. However, in polar semiconductors, the Fröhlich electron-phonon coupling is strong and its influence on phononic thermal transport is of great significance. In this work, the effect of EPI on phonon dispersion and lattice thermal conductivity of wurtzite gallium nitride (GaN) is comprehensively investigated from the atomistic level by performing first-principles calculations. Due to the existence of relatively large electronegativity difference between Ga and N atoms, the Fröhlich coupling in wurtzite GaN is remarkably strong. Consequently, the lattice thermal conductivity of natural wurtzite GaN at room temperature is reduced by ˜24%-34% when including EPI, and the resulted thermal conductivity value is in better agreement with experiments. Furthermore, the scattering rate of phonons due to EPI, the intrinsic phonon-phonon interaction (PPI) as well as isotope disorder is computed and analyzed. It shows that the EPI scattering rate is comparable to PPI for low-frequency heat-carrying phonons. This work attempts to explore the mechanism of thermal transport beyond intrinsic PPI for polar semiconductors, with a great potential of thermal conductivity engineering for desired performance.

  14. Phonon quarticity induced by changes in phonon-tracked hybridization during lattice expansion and its stabilization of rutile TiO2

    SciTech Connect

    Lan, Tian; Li, Chen W.; Hellman, O.; Kim, D. S.; Muñoz, Jorge A.; Smith, Hillary; Abernathy, Douglas L.; Fultz, B.

    2015-08-11

    Although the rutile structure of TiO2 is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly predicting a structural collapse at temperatures well below 1000 K. In this paper, inelastic neutron scattering was used to measure the temperature dependence of the phonon density of states (DOS) of rutile TiO2 from 300 to 1373 K. Surprisingly, these anomalous acoustic phonons were found to increase in frequency with temperature. First-principles calculations showed that with lattice expansion, the potentials for the anomalous acoustic phonons transform from quadratic to quartic, stabilizing the rutile phase at high temperatures. In these modes, the vibrational displacements of adjacent Ti and O atoms cause variations in hybridization of 3d electrons of Ti and 2p electrons of O atoms. Finally, with thermal expansion, the energy variation in this “phonon-tracked hybridization” flattens the bottom of the interatomic potential well between Ti and O atoms, and induces a quarticity in the phonon potential.

  15. Comparing the anomalous phonons in Fe(Te,Se) and (Fe,Ni)(Te,Se) via neutron scattering

    NASA Astrophysics Data System (ADS)

    Schneeloch, John; Xu, Zhijun; Gu, Genda; Zaliznyak, Igor; Winn, Barry; Rodriguez-Rivera, Jose; Birgeneau, Robert; Xu, Guangyong; Tranquada, John

    We studied the anomalous acoustic-type phonons in the Fe(Te,Se) iron-based superconductor family that arise from the (100) Bragg peak, which is forbidden according to the reported crystal structure for these materials. Inelastic neutron scattering was performed on superconducting and non-superconducting crystals of various compositions. The (100) phonons were much weaker in a non-superconducting nickel-doped crystal than in a superconducting crystal with similar selenium fraction, but comparison with another non-superconducting crystal suggests the difference is not simply related to superconductivity. This composition dependence was observed for both transverse and longitudinal phonons. The temperature dependences of the (100) phonons resembled those of conventional phonons. We will discuss these results and possible explanations for the relation between composition and lattice dynamics in this system.

  16. Anomalous Infrared Spectra of Hybridized Phonons in Type-I Clathrate Ba8Ga16Ge30

    NASA Astrophysics Data System (ADS)

    Iwamoto, Kei; Kushibiki, Shunsuke; Honda, Hironori; Kajitani, Shuhei; Mori, Tatsuya; Matsumoto, Hideki; Toyota, Naoki; Suekuni, Koichiro; Avila, Marcos A.; Takabatake, Toshiro

    2013-02-01

    The optical conductivity spectra of the rattling phonons in the clathrate Ba8Ga16Ge30 are investigated in detail by use of the terahertz time-domain spectroscopy. The experiment has revealed that the lowest-lying vibrational mode of Ba(2)2+ ions consist of a sharp Lorentzian peak at 1.2 THz superimposed on a broad tail weighted in the lower frequency regime around 1.0 THz. With decreasing temperature, an unexpected linewidth broadening of the phonon peak is observed, together with monotonic softening of the phonon peak and enhancement of the tail structure. These observed anomalies are discussed in terms of impurity scattering effects on the hybridized phonon system of rattling and acoustic phonons.

  17. Phonon-drag thermopower and hot-electron energy-loss rate in a Rashba spin-orbit coupled two-dimensional electron system.

    PubMed

    Biswas, Tutul; Ghosh, Tarun Kanti

    2013-07-03

    We theoretically study the phonon-drag contribution to the thermoelectric power and the hot-electron energy-loss rate in a Rashba spin-orbit coupled two-dimensional electron system in the Bloch-Gruneisen (BG) regime. We assume that electrons interact with longitudinal acoustic phonons through a deformation potential and with both longitudinal and transverse acoustic phonons through a piezoelectric potential. The effect of the Rashba spin-orbit interaction on the magnitude and temperature dependence of the phonon-drag thermoelectric power and hot-electron energy-loss rate is discussed. We numerically extract the exponent of temperature dependence of the phonon-drag thermopower and the energy-loss rate. We find that the exponents are suppressed due to the presence of the Rashba spin-orbit coupling.

  18. Spectral phonon mean free path and thermal conductivity accumulation in defected graphene: The effects of defect type and concentration

    NASA Astrophysics Data System (ADS)

    Feng, Tianli; Ruan, Xiulin; Ye, Zhenqiang; Cao, Bingyang

    2015-06-01

    The spectral phonon properties in defected graphene have been unclear due to the lack of advanced techniques for predicting the phonon-defect scattering rate without fitting parameters. Taking advantage of the extended phonon normal mode analysis, we obtained the spectral phonon relaxation time and mean free path (MFP) in defected graphene and studied the impacts of three common types of defects: Stone-Thrower-Wales (STW) defect, double vacancy (DV), and monovacancy (MV). The phonon-STW defect scattering rate is found to have no significant frequency dependence, and as a result, the relative contribution of long-wavelength phonons sharply decreases. In contrast, the phonon scattering by DVs or MVs exhibits a frequency dependence of τp-d -1˜ω1.1 -1.3 except for a few long-wavelength phonons, revisiting the traditionally used ˜ω4 dependence. We note that although MV-defected graphene has the lowest thermal conductivity as compared to the other two defected graphene samples at the same defect concentration, it has a portion of phonons with the longest MFP. The contribution from the long-MFP and long-wavelength phonons does not decrease much as the vacancy concentration increases. STW defect and MV block more out-of-plane modes than in-plane modes, while DV has less bias for which mode to block. As the MV concentration increases from 0 to 1.1%, the relative contribution from out-of-plane modes decreases from 30% to 18%, while that of the transverse acoustic mode remains at around 30%. These findings of spectral phonon properties can provide more insight than the effective properties and benefit the prospective phononic engineering.

  19. Direct measurement of lattice dynamics and optical phonon excitation in semiconductor nanocrystals using femtosecond stimulated Raman spectroscopy.

    PubMed

    Hannah, Daniel C; Brown, Kristen E; Young, Ryan M; Wasielewski, Michael R; Schatz, George C; Co, Dick T; Schaller, Richard D

    2013-09-06

    We report femtosecond stimulated Raman spectroscopy measurements of lattice dynamics in semiconductor nanocrystals and characterize longitudinal optical (LO) phonon production during confinement-enhanced, ultrafast intraband relaxation. Stimulated Raman signals from unexcited CdSe nanocrystals produce a spectral shape similar to spontaneous Raman signals. Upon photoexcitation, stimulated Raman amplitude decreases owing to experimentally resolved ultrafast phonon generation rates within the lattice. We find a ∼600  fs, particle-size-independent depletion time attributed to hole cooling, evidence of LO-to-acoustic down-conversion, and LO phonon mode softening.

  20. Nonmonotonic Diameter Dependence of Thermal Conductivity of Extremely Thin Si Nanowires: Competition between Hydrodynamic Phonon Flow and Boundary Scattering.

    PubMed

    Zhou, Yanguang; Zhang, Xiaoliang; Hu, Ming

    2017-02-08

    By carefully and systematically performing Green-Kubo equilibrium molecular dynamics simulations, we report that the thermal conductivity (κ) of Si nanowires (NWs) does not diverge but converges and increases steeply when NW diameter (D) becomes extremely small (dκ/dD < 0), a long debate of one-dimensional heat conduction in history. The κ of the thinnest possible Si NWs reaches a superhigh level that is as large as more than 1 order of magnitude higher than its bulk counterpart. The abnormality is explained in terms of the dominant normal (N) process (energy and momentum conservation) of low frequency acoustic phonons that induces hydrodynamic phonon flow in the Si NWs without being scattered. With D increasing, the downward shift of optical phonons triggers strong Umklapp (U) scattering with acoustic phonons and attenuates the N process, leading to the regime of phonon boundary scattering (dκ/dD < 0). The two competing mechanisms result in nonmonotonic diameter dependence of κ with minima at critical diameter of 2-3 nm. Our results unambiguously demonstrate the converged κ and the clear trend of κ ∼ D for extremely thin Si NWs by fully elucidating the competition between the hydrodynamic phonon flow and phonon boundary scattering.

  1. Lamb wave band gaps in one-dimensional radial phononic crystal slabs

    NASA Astrophysics Data System (ADS)

    Li, Yinggang; Chen, Tianning; Wang, Xiaopeng

    2015-10-01

    In this paper, we theoretically investigate the band structures of Lamb wave in one-dimensional radial phononic crystal (PC) slabs composed of a series of alternating strips of epoxy and aluminum. The dispersion relations, the power transmission spectra and the displacement fields of the eigenmodes are calculated by using the finite element method based on two-dimensional axial symmetry models in cylindrical coordinates. The axial symmetry model is validated by three-dimensional finite element model in Cartesian coordinates. Numerical results show that the proposed radial PC slabs can yield several complete band gaps with a variable bandwidth exist for elastic waves. Furthermore, the effects of the filling fraction and the slab thickness on the band gaps are further explored numerically. It is worth observing that, with the increase of the filling fraction, both the lower and upper edges of the band gaps are simultaneously shifted to higher frequency, which results from the enhancement interaction between the rigid resonance of the scatterer and the matrix. The slab thickness is the key parameter for the existence and the width of complete band gaps in the radial PC slabs. These properties of Lamb waves in the radial PC plates can potentially be applied to optimize band gaps, generate filters and design acoustic devices in the rotary machines and structures.

  2. Neutron Scattering Investigation of Phonon Scattering Rates in Ag1-xSb1+xTe2+x (x = 0, 0.1, and 0.2)

    SciTech Connect

    Abernathy, Douglas L; Budai, John D; Delaire, Olivier A; Ehlers, Georg; Hong, Tao; Karapetrova, Evguenia A.; Ma, Jie; May, Andrew F; McGuire, Michael A; Specht, Eliot D

    2014-01-01

    The phonon dispersions and scattering rates of the thermoelectric material AgSbTe$_{2}$ were measured as a function of temperature with inelastic neutron scattering. The results show that phonon scattering rates are large and weakly dependent on temperature. The lattice thermal conductivity was calculated from the measured phonon lifetimes and group velocities, providing good agreement with bulk transport measurements. The measured phonon scattering rates and their temperature dependence are compared with models of phonon scattering by anharmonicity and point defect. We find that these processes cannot account for the large total phonon scattering rates observed, and their lack of temperature dependence. Neutron and synchrotron diffraction measurements on single crystals revealed an extensive nanostructure from cation ordering, which is likely responsible for the strong phonon scattering.

  3. Phonons and hybrid modes in the high and low temperature far infrared dynamics of hexagonal TmMnO3.

    PubMed

    Massa, Néstor E; del Campo, Leire; De Sousa Meneses, Domingos; Echegut, Patrick; Martínez-Lope, María Jesús; Alonso, José Antonio

    2014-07-09

    We report on temperature dependent TmMnO3 far infrared emissivity and reflectivity spectra from 1910 K to 4 K. At the highest temperature the number of infrared bands is lower than that predicted for centrosymmetric P63/mmc (D(4)(6h)) (Z = 2) space group due to high temperature anharmonicity and possible defect induced bitetrahedra misalignments. On cooling, at ~1600 ± 40 K, TmMnO3 goes from non-polar to an antiferroelectric-ferroelectric polar phase reaching the ferroelectric onset at ~700 K. Room temperature reflectivity is fitted using 19 oscillators and this number of phonons is maintained down to 4 K. A weak phonon anomaly in the band profile at 217 cm(-1) (4 K) suggests subtle Rare Earth magneto-electric couplings at ~TN and below. A low energy collective excitation is identified as a THz instability associated with room temperature eg electrons in a d-orbital fluctuating environment. It condenses into two modes that emerge pinned to the E-type antiferromagnetic order hardening simultaneously down to 4 K. They obey power laws with TN as the critical temperature and match known zone center magnons. The one peaking at 26 cm(-1), with critical exponent β=0.42 as for antiferromagnetic order in a hexagonal lattice, is dependent on the Rare Earth ion. The higher frequency companion at ~50 cm(-1), with β=0.25, splits at ~TN into two peaks. The weaker band of the two is assimilated to the upper branch of the gap opening in the transverse acoustical (TA) phonon branch crossing the magnetic dispersion found in YMnO3. (Petit et al 2007 Phys. Rev. Lett. 99 266604). The stronger second band at ~36 cm(-1) corresponds to the lower branch of the TA gap. We assign both excitations as zone center magneto-electric hybrid quasiparticles, concluding that in NdMnO3 perovskite the equivalent picture corresponds to an instability which may be driven by an external field to transform NdMnO3 into a multiferroic compound by perturbation enhancing the TA

  4. Determination of symmetry reduced structures using a soft phonon analysis for magnetic shape memory alloys (abstract only).

    PubMed

    Hickel, Tilmann; Uijttewaal, Matthé; Grabowski, Blazej; Neugebauer, Jörg

    2008-02-13

    Ni(2)MnGa is a typical example of a Heusler alloy that undergoes a martensitic transformation. In the high temperature austenitic phase it has a cubic L2(1) structure, whereas below 200 K the symmetry is reduced by an orthorhombic distortion. Despite lattice deformations of more than 6% and large strains connected to this change, it is completely reversible. Therefore, Ni(2)MnGa serves as a shape memory compound. The fact that Ni(2)MnGa additionally orders ferromagnetically below 360 K makes the material particularly attractive for applications in actuators and sensors. Nevertheless, its structural details in the martensitic phase are still a subject of much debate. Several shuffling structures have been observed experimentally. The temperature and magnetic field dependent transformations between these structures need to be understood for improvement of the magnetic switching (e.g. operation with higher reliability and smaller magnetic fields). Our tool for identifying the stable structures and the low energy transition paths is the calculation of free energy surfaces as functions of key reaction coordinates (e.g. the ratio c/a) in density functional theory. (The generalized gradient approximation to the exchange-correlation functional and the projector augmented wave approach implemented in VASP (Vienna Ab initio Simulation Package) were used in these investigations.) The different variants of the low symmetry orthorhombic structures lead to characteristic minima on this surface. However, the ab initio determination of the experimentally observed shuffling structures is challenging, due to the large phase space of possible atomic positions and the small shuffling formation energies of only a few meV per unit cell. Hence, we used the quasiharmonic approximation in order to compute and analyze phonon spectra. Starting with the symmetric structure of the austenite, the TA(2) (TA standing for transverse acoustic) phonon dispersion shows a phonon softening along

  5. Band structures in the nematic elastomers phononic crystals

    NASA Astrophysics Data System (ADS)

    Yang, Shuai; Liu, Ying; Liang, Tianshu

    2017-02-01

    As one kind of new intelligent materials, nematic elastomers (NEs) represent an exciting physical system that combines the local orientational symmetry breaking and the entropic rubber elasticity, producing a number of unique physical phenomena. In this paper, the potential application of NEs in the band tuning is explored. The band structures in two kinds of NE phononic crystals (PCs) are investigated. Through changing NE intrinsic parameters, the influence of the porosity, director rotation and relaxation on the band structures in NE PCs are analyzed. This work is a meaningful try for application of NEs in acoustic field and proposes a new intelligent strategy in band turning.

  6. Helium Atom Scattering as a Probe of Surface Phonons.

    NASA Astrophysics Data System (ADS)

    Yerkes, Steven Charles

    A low energy (15-63 meV) helium beam is scattered from two different crystal surfaces; mechanically cleaved and polished LiF(100), and epitaxially grown Ag(111). Conservation equations for total particle energy and parallel momentum are presented as the basis for understanding the scattering experiment. These equations along with the system response function are used to numerically model the inelastic scattering data. The scattering of helium from LiF(100) at a surface temperature of approximately 140(DEGREES)K is reported along the <010> and <110> directions. Coherent elastic scattering intensities are used for surface characterization. Over 80% of the coherent inelastic scattering can be accounted for by the interaction with single Rayleigh phonons, and is consistent with a calculated rigid-ion Rayleigh phonon dispersion relation of LiF(100). These conclusions are supported by over 85 separate inelastic experiments performed at two incident beam energies (62.5 meV and 20.5 meV) and at several incident angles (50(DEGREES), 60(DEGREES), 65(DEGREES), 70(DEGREES)). The scattering from single Rayleigh phonons is reported as a function of crystal surface temperature, scattering angle, phonon frequency, and azimuthal angle. The inelastic scattering data is compared with the calculated intensities of an analytic inelastic scattering theory. The surface temperature dependent inelastic scattering intensity of the data are qualitatively predicted by the theory, however, the theory is inadequate in predicting the experimental intensity as a function of scattering angle, phonon frequency, and azimuthal angle. Incoherent elastic scattering (due to surface defects) is also reported as a function of scattered angle. No existing theory can account for the observed behavior of this scattering. Preliminary coherent inelastic scattering data are reported for. 23 meV helium from Ag(111) directed 12.5(DEGREES) from the <112>. Single(' ). Rayleigh phonons account for less than 60% of

  7. Acoustic Neuroma

    MedlinePlus

    ... search IRSA's site Unique Hits since January 2003 Acoustic Neuroma Click Here for Acoustic Neuroma Practice Guideline ... to microsurgery. One doctor's story of having an acoustic neuroma In August 1991, Dr. Thomas F. Morgan ...

  8. Phonon transport in single-layer boron nanoribbons

    NASA Astrophysics Data System (ADS)

    Zhang, Zhongwei; Xie, Yuee; Peng, Qing; Chen, Yuanping

    2016-11-01

    Inspired by the successful synthesis of three two-dimensional (2D) allotropes, the boron sheet has recently been one of the hottest 2D materials around. However, to date, phonon transport properties of these new materials are still unknown. By using the non-equilibrium Green’s function (NEGF) combined with the first principles method, we study ballistic phonon transport in three types of boron sheets; two of them correspond to the structures reported in the experiments, while the third one is a stable structure that has not been synthesized yet. At room temperature, the highest thermal conductance of the boron nanoribbons is comparable with that of graphene, while the lowest thermal conductance is less than half of graphene’s. Compared with graphene, the three boron sheets exhibit diverse anisotropic transport characteristics. With an analysis of phonon dispersion, bonding charge density, and simplified models of atomic chains, the mechanisms of the diverse phonon properties are discussed. Moreover, we find that many hybrid patterns based on the boron allotropes can be constructed naturally without doping, adsorption, and defects. This provides abundant nanostructures for thermal management and thermoelectric applications.

  9. Optical phonons in PbTe/CdTe multilayer heterostructures

    SciTech Connect

    Novikova, N. N.; Yakovlev, V. A.; Kucherenko, I. V.; Karczewski, G.; Aleshchenko, Yu. A.; Muratov, A. V.; Zavaritskaya, T. N.; Melnik, N. N.

    2015-05-15

    The infrared reflection spectra of PbTe/CdTe multilayer nanostructures grown by molecular-beam epitaxy are measured in the frequency range of 20–5000 cm{sup −1} at room temperature. The thicknesses and high-frequency dielectric constants of the PbTe and CdTe layers and the frequencies of the transverse optical (TO) phonons in these structures are determined from dispersion analysis of the spectra. It is found that the samples under study are characterized by two TO phonon frequencies, equal to 28 and 47 cm{sup −1}. The first frequency is close to that of TO phonons in bulk PbTe, and the second is assigned to the optical mode in structurally distorted interface layers. The Raman-scattering spectra upon excitation with the radiation of an Ar{sup +} laser at 514.5 nm are measured at room and liquid-nitrogen temperatures. The weak line at 106 cm{sup −1} observed in these spectra is attributed to longitudinal optical phonons in the interface layers.

  10. Scattering of phonons by vacancies

    SciTech Connect

    Ratsifaritana, C.A.; Klemens, P.G.

    1987-11-01

    The scattering of phonons by vacancies is estimated by a perturbation technique in terms of the missing mass and the missing linkages. An argument is given why distortion effects can be disregarded. The resonance frequency of the defect is sufficiently high so that resonance effects can be disregarded for phonons in the important frequency range for thermal conduction. The theory is applied to the thermal resistance by vacancies in cases where the vacancy concentration is known: potassium chloride with divalent cations, nonstoichiometric zirconium carbide, and tin telluride.

  11. Prospective Assessment of Correlation between US Acoustic Radiation Force Impulse and MR Elastography in a Pediatric Population: Dispersion of US Shear-Wave Speed Measurement Matters.

    PubMed

    Trout, Andrew T; Dillman, Jonathan R; Xanthakos, Stavra; Kohli, Rohit; Sprague, Garrett; Serai, Suraj; Mahley, Alana D; Podberesky, Daniel J

    2016-11-01

    Purpose To evaluate the correlation between ultrasonographic (US) point shear-wave elastography (SWE) and magnetic resonance (MR) elastography liver shear-wave speed (SWS) measurements in a pediatric population and to determine if US data dispersion affects this relationship. Materials and Methods Institutional review board approval was obtained for this HIPAA-compliant investigation; informed consent and patient assent (as indicated) were obtained. Patients (age range, 0-21 years) undergoing clinical liver MR elastography between July 2014 and November 2015 were prospectively enrolled. Patients underwent two-dimensional gradient-recalled-echo 1.5-T MR elastography with point SWE performed immediately before or immediately after MR elastography. Spearman rank correlation coefficients were calculated to assess the relationship and agreement between point SWE and MR elastography SWS measurements. Uni- and multivariate logistic regression were performed to identify predictors of US data dispersion, with the best multivariate model selected based on Akaike information criterion. Results A total of 55 patients (24 female) were enrolled (mean age, 14.0 years ± 3.9 (standard deviation) (range, 3.5-21.4 years). There was fair correlation between point SWE and MR elastography SWS values for all patients (ρ = 0.33, P = .016). Correlation was substantial, however, when including only patients with minimal US data dispersion (n = 26, ρ = 0.61, P = .001). Mean body mass index (BMI) was significantly lower in patients with minimal US data dispersion than in those with substantial US data dispersion (25.4 kg/m(2) ± 7.8 vs 32.3 kg/m(2) ± 8.3, P = .003). At univariate analysis, BMI (odds ratio, 1.12; 95% confidence interval [CI]: 1.03, 1.21; P = .006) and abdominal wall thickness (odds ratio, 2.50; 95% CI: 1.32, 4.74; P = .005) were significant predictors of US data dispersion. In the best multivariate model, BMI was the only significant predictor (odds ratio, 1.11; 95% CI: 1

  12. Generation and detection of incoherent phonons in picosecond ultrasonics.

    PubMed

    Perrin, B; Péronne, E; Belliard, L

    2006-12-22

    In picosecond ultrasonics experiments the absorption of a femtosecond laser pulse in a thin metallic transducer is used to generate very short acoustic pulses. These pulses are made of coherent longitudinal waves with a frequency spectrum that can reach 100-200 GHz. The laser pulse absorption gives rise to a heating of the film of a few Kelvin within a typical time of 1 ps. Later on, the heat goes in the substrate through an interface thermal resistance and is diffused by thermal conduction. At very low temperature and in pure crystals the thermal phonons emitted by the heated metallic film can propagate ballistically over large distances and produce a so-called heat pulse. We report on the experimental evidence of the coexistence of the coherent acoustic pulse and the incoherent heat pulse generated and detected by laser ultrasonics.

  13. The effects of substrate phonon mode scattering on transport in carbon nanotubes.

    PubMed

    Perebeinos, Vasili; Rotkin, Slava V; Petrov, Alexey G; Avouris, Phaedon

    2009-01-01

    Carbon nanotubes (CNTs) have large intrinsic carrier mobility due to weak acoustic phonon scattering. However, unlike two-dimensional metal-oxide-semiconductor field effect transistors (MOSFETs), substrate surface polar phonon (SPP) scattering has a dramatic effect on the CNTFET mobility, due to the reduced vertical dimensions of the latter. We find that for the van der Waals distance between CNT and an SiO2 substrate, the low-field mobility at room temperature is reduced by almost an order of magnitude depending on the tube diameter. We predict additional experimental signatures of the SPP mechanism in dependence of the mobility on density, temperature, tube diameter, and CNT-substrate separation.

  14. Electron-phonon interaction and Raman scattering in nanocrystals

    NASA Astrophysics Data System (ADS)

    Klimin, S. N.; Pokatilov, E. P.; Fomin, V. M.; Devreese, J. T.; Gladilin, V. N.; Balaban, S. N.

    1997-03-01

    The vibrational eigenmodes of a nanocrystal are derived by diagonalization of the equations of motion for the ionic displacement taking into account a non-parabolic dispersion with electrostatic and mechanical boundary conditions. A finite width of the Brillouin zone leads automatically to a finite basis of vibrational modes. The developed method can be applicable to nanostructures of an arbitrary geometry. For a spherical nanocrystal, a dispersion equation contains the effective multimode dielectric function. The resulting eigenmodes are mixed bulk-like and interface waves, especially in the short-wavelength region. Using the obtained Hamiltonian, the one-phonon and two-phonon resonant Raman scattering spectra are calculated for a spherical CdSe nanocrystal in the borosilicate glass. The valence band mixing dramatically enhances relative intensities of the two-phonon peaks and makes the adiabatic approximation inapplicable. Hence, the Huang-Rhys parameter is not an adequate characteristic of the optical spectra. Using a direct expansion of the evolution operator, a good agreement has been achieved between the calculated and the experimentally observed [1] Raman spectra. [1] M. C. Klein, F. Hache, D. Ricard, and C. Flytzanis, Phys. Rev. B 42, 11123 (1990).

  15. Phonon density of states of Sn in textured SnO under high pressure: Comparison of nuclear inelastic x-ray scattering spectra to a shell model

    NASA Astrophysics Data System (ADS)

    Giefers, H.; Koval, S.; Wortmann, G.; Sturhahn, W.; Alp, E. E.; Hu, M. Y.

    2006-09-01

    The local phonon density of states (DOS) at the Sn site in tin monoxide (SnO) is studied at pressures up to 8GPa with Sn119 nuclear resonant inelastic x-ray scattering (NRIXS) of synchrotron radiation at 23.88keV . The preferred orientation (texture) of the SnO crystallites in the investigated samples is used to measure NRIXS spectra preferentially parallel and almost perpendicular to the c axis of tetragonal SnO . A subtraction method is applied to these NRIXS spectra to produce projected local Sn DOS spectra as seen parallel and perpendicular to the c axis of SnO . These experimentally obtained local Sn DOS spectra, both in the polycrystalline case as well as projected parallel and perpendicular to the c axis, are compared with corresponding theoretical phonon DOS spectra, derived from dispersion relations calculated with a recently developed shell model. Comparison between the experimental projected Sn DOS spectra and the corresponding theoretical DOS spectra enables us to follow the pressure-induced shifts of several acoustic and optic phonon modes. While the principal spectral features of the experimental and theoretical phonon DOS agree well at energies above 10meV , the pressure behavior of the low-energy part of the DOS is not well reproduced by the theoretical calculations. In fact, they exhibit, in contrast to the experimental data, a dramatic softening of two low-energy modes, their energies approaching zero around 2.5GPa , clearly indicating the limitations of the applied shell model. These difficulties are obviously connected with the complex Sn-O and Sn-Sn bindings within and between the Sn-O-Sn layers in the litharge structure of SnO . We derived from the experimental and theoretical DOS spectra a variety of elastic and thermodynamic parameters of the Sn sublattice, such as the Lamb-Mössbauer factor, the mean force constant, and Debye temperatures, as well as the vibrational contributions to the Helmholtz free energy, specific heat, entropy, and

  16. Current & Heat Transport in Graphene Nanoribbons: Role of Non-Equilibrium Phonons

    NASA Astrophysics Data System (ADS)

    Pennington, Gary; Finkenstadt, Daniel

    2010-03-01

    The conducting channel of a graphitic nanoscale device is expected to experience a larger degree of thermal isolation when compared to traditional inversion channels of electronic devices. This leads to enhanced non-equilibrium phonon populations which are likely to adversely affect the mobility of graphene-based nanoribbons due to enhanced phonon scattering. Recent reports indicating the importance of carrier scattering with substrate surface polar optical phonons in carbon nanotubes^1 and graphene^2,3 show that this mechanism may allow enhanced heat removal from the nanoribbon channel. To investigate the effects of hot phonon populations on current and heat conduction, we solve the graphene nanoribbon multiband Boltzmann transport equation. Monte Carlo transport techniques are used since phonon populations may be tracked and updated temporally.^4 The electronic structure is solved using the NRL Tight-Binding method,^5 where carriers are scattered by confined acoustic, optical, edge and substrate polar optical phonons. [1] S. V. Rotkin et al., Nano Lett. 9, 1850 (2009). [2] J. H. Chen, C. Jang, S. Xiao, M. Ishigami and M. S. Fuhrer, Nature Nanotech. 3, 206 (2008). [3] V. Perebeinos and P. Avouris, arXiv:0910.4665v1 [cond-mat.mes-hall] (2009). [4] P. Lugli et al., Appl. Phys. Lett. 50, 1251 (1987). [5] D. Finkenstadt, G. Pennington & M.J. Mehl, Phys. Rev. B 76, 121405(R) (2007).

  17. Nanoscale transport of phonons: Dimensionality, subdiffusion, molecular damping, and interference effects

    SciTech Connect

    Walczak, Kamil; Yerkes, Kirk L.

    2014-05-07

    We examine heat transport carried by acoustic phonons in the systems composed of nanoscale chains of masses coupled to two thermal baths of different temperatures. Thermal conductance is obtained by using linearized Landauer-type formula for heat flux with phonon transmission probability calculated within atomistic Green's functions (AGF) method. AGF formalism is extended onto dissipative chains of masses with harmonic coupling beyond nearest-neighbor approximation, while atomistic description of heat reservoirs is also included into computational scheme. In particular, the phonon lifetimes and the phonon frequency shifts are discussed for harmonic lattices of different dimensions. Further, resonant structure of phonon transmission spectrum is analyzed with respect to reservoir-induced effects, molecular damping, and mass-to-mass harmonic coupling. Analysis of transmission zeros (antiresonances) and their accompanied Fano-shape resonances are discussed as a result of interference effects between different vibrational modes. Finally, we also predict subdiffusive transport regime for low-frequency ballistic phonons propagated along a linear chain of harmonically coupled masses.

  18. Nanoscale transport of phonons: Dimensionality, subdiffusion, molecular damping, and interference effects

    NASA Astrophysics Data System (ADS)

    Walczak, Kamil; Yerkes, Kirk L.

    2014-05-01

    We examine heat transport carried by acoustic phonons in the systems composed of nanoscale chains of masses coupled to two thermal baths of different temperatures. Thermal conductance is obtained by using linearized Landauer-type formula for heat flux with phonon transmission probability calculated within atomistic Green's functions (AGF) method. AGF formalism is extended onto dissipative chains of masses with harmonic coupling beyond nearest-neighbor approximation, while atomistic description of heat reservoirs is also included into computational scheme. In particular, the phonon lifetimes and the phonon frequency shifts are discussed for harmonic lattices of different dimensions. Further, resonant structure of phonon transmission spectrum is analyzed with respect to reservoir-induced effects, molecular damping, and mass-to-mass harmonic coupling. Analysis of transmission zeros (antiresonances) and their accompanied Fano-shape resonances are discussed as a result of interference effects between different vibrational modes. Finally, we also predict subdiffusive transport regime for low-frequency ballistic phonons propagated along a linear chain of harmonically coupled masses.

  19. Giant phonon anomaly associated with superconducting fluctuations in the pseudogap phase of cuprates

    DOE PAGES

    Liu, Ye-Hua; Konik, Robert M.; Rice, T. M.; ...

    2016-01-20

    The pseudogap in underdoped cuprates leads to significant changes in the electronic structure, and was later found to be accompanied by anomalous fluctuations of superconductivity and certain lattice phonons. Here we propose that the Fermi surface breakup due to the pseudogap, leads to a breakup of the pairing order into two weakly coupled sub-band amplitudes, and a concomitant low energy Leggett mode due to phase fluctuations between them. This increases the temperature range of superconducting fluctuations containing an overdamped Leggett mode. In this range inter-sub-band phonons show strong damping due to resonant scattering into an intermediate state with a pairmore » of overdamped Leggett modes. In the ordered state, the Leggett mode develops a finite energy, changing the anomalous phonon damping into an anomaly in the dispersion. Finally, this proposal explains the intrinsic connection between the anomalous pseudogap phase, enhanced superconducting fluctuations and giant anomalies in the phonon spectra.« less

  20. Giant phonon anomaly associated with superconducting fluctuations in the pseudogap phase of cuprates

    PubMed Central

    Liu, Ye-Hua; Konik, Robert M.; Rice, T. M.; Zhang, Fu-Chun

    2016-01-01

    The pseudogap in underdoped cuprates leads to significant changes in the electronic structure, and was later found to be accompanied by anomalous fluctuations of superconductivity and certain lattice phonons. Here we propose that the Fermi surface breakup due to the pseudogap, leads to a breakup of the pairing order into two weakly coupled sub-band amplitudes, and a concomitant low energy Leggett mode due to phase fluctuations between them. This increases the temperature range of superconducting fluctuations containing an overdamped Leggett mode. In this range inter-sub-band phonons show strong damping due to resonant scattering into an intermediate state with a pair of overdamped Leggett modes. In the ordered state, the Leggett mode develops a finite energy, changing the anomalous phonon damping into an anomaly in the dispersion. This proposal explains the intrinsic connection between the anomalous pseudogap phase, enhanced superconducting fluctuations and giant anomalies in the phonon spectra. PMID:26785835