Temperature dependence of the LO phonon sidebands in free exciton emission of GaN
NASA Astrophysics Data System (ADS)
Xu, S. J.; Li, G. Q.; Xiong, S.-J.; Che, C. M.
2006-04-01
Temperature-dependent radiative recombination of free excitons involving one or two LO phonons in GaN is investigated in detail. It is found that both phonon sidebands possess asymmetric lineshapes and their energy spacings from the zero-phonon line strongly deviate from the characteristic energy of LO phonons as the temperature increases. Furthermore, the deviation rates of one- and two-phonon sidebands are significantly different. Segall-Mahan [Phys. Rev. 171, 935 (1968)] theory, taking the exciton-photon and exciton-phonon interactions into account, is employed to calculate the sidebands of one or two LO phonons for free excitons in a wide temperature range. Excellent agreement between the theory and experiment is achieved by using only one adjustable parameter, which leads to determination of the effective mass of heavy holes (~0.5m0).
Resolved-sideband Raman cooling of an optical phonon in semiconductor materials
NASA Astrophysics Data System (ADS)
Zhang, Jun; Zhang, Qing; Wang, Xingzhi; Kwek, Leong Chuan; Xiong, Qihua
2016-09-01
The radiation pressure of light has been widely used to cool trapped atoms or the mechanical vibrational modes of optomechanical systems. Recently, by using the electrostrictive forces of light, spontaneous Brillouin cooling and stimulated Brillouin excitation of acoustic modes of the whispering-gallery-type resonator have been demonstrated. The laser cooling of specific lattice vibrations in solids (that is, phonons) proposed by Dykman in the late 1970s, however, still remains sparsely investigated. Here, we demonstrate the first strong spontaneous Raman cooling and heating of a longitudinal optical phonon (LOP) with a 6.23 THz frequency in polar semiconductor zinc telluride nanobelts. We use the exciton to resonate and assist photoelastic Raman scattering from the LOPs caused by a strong exciton-LOP coupling. By detuning the laser pump to a lower (higher) energy-resolved sideband to make a spontaneous scattering photon resonate with an exciton at an anti-Stokes (Stokes) frequency, the dipole oscillation of the LOPs is photoelastically attenuated (enhanced) to a colder (hotter) state.
Zhao, Hong-Quan; Fujiwara, Masazumi; Takeuchi, Shigeki
2012-07-02
Substrates effect is observed on the suppression of the phonon sideband from nitrogen vacancy (NV) centers in 50nm diamond nanocrystals at cryogenic temperatures. As a quantitative parameter of the population of phonon sidebands, the Debye-Waller factor is estimated from fluorescence spectra on glass, silicon, and silica-on-silicon substrates. Fluorescence spectra of negatively charged NV centers in nanodiamonds on silica-on-silicon substrates have average and maximum Debye-Waller factors of 12.7% (which is about six times greater than that of samples on glass substrates) and 19.3%, respectively. This effect is expected to be very important for future applications of NV centers in quantum information science and nanosensing.
Acoustic superfocusing by solid phononic crystals
Zhou, Xiaoming; Assouar, M. Badreddine Oudich, Mourad
2014-12-08
We propose a solid phononic crystal lens capable of acoustic superfocusing beyond the diffraction limit. The unit cell of the crystal is formed by four rigid cylinders in a hosting material with a cavity arranged in the center. Theoretical studies reveal that the solid lens produces both negative refraction to focus propagating waves and surface states to amplify evanescent waves. Numerical analyses of the superfocusing effect of the considered solid phononic lens are presented with a separated source excitation to the lens. In this case, acoustic superfocusing beyond the diffraction limit is evidenced. Compared to the fluid phononic lenses, the solid lens is more suitable for ultrasonic imaging applications.
Acoustic superfocusing by solid phononic crystals
NASA Astrophysics Data System (ADS)
Zhou, Xiaoming; Assouar, M. Badreddine; Oudich, Mourad
2014-12-01
We propose a solid phononic crystal lens capable of acoustic superfocusing beyond the diffraction limit. The unit cell of the crystal is formed by four rigid cylinders in a hosting material with a cavity arranged in the center. Theoretical studies reveal that the solid lens produces both negative refraction to focus propagating waves and surface states to amplify evanescent waves. Numerical analyses of the superfocusing effect of the considered solid phononic lens are presented with a separated source excitation to the lens. In this case, acoustic superfocusing beyond the diffraction limit is evidenced. Compared to the fluid phononic lenses, the solid lens is more suitable for ultrasonic imaging applications.
Depth-Dependent Defect Studies Using Coherent Acoustic Phonons
2014-09-29
12211 Research Triangle Park, NC 27709-2211 coherent acoustic phonons, diamond, silicon, photelastic coefficients , refractive index, graphene, Second...attributed to the cooling of the subsystem of hot optical phonons by optical- acoustic phonon scattering . We observe that at different pump energy and...SECURITY CLASSIFICATION OF: Presented is our scientific progress in two areas of research. The first is coherent acoustic phonon (CAP) spectroscopy of
Yudistira, D; Boes, A; Djafari-Rouhani, B; Pennec, Y; Yeo, L Y; Mitchell, A; Friend, J R
2014-11-21
We theoretically and experimentally demonstrate the existence of complete surface acoustic wave band gaps in surface phonon-polariton phononic crystals, in a completely monolithic structure formed from a two-dimensional honeycomb array of hexagonal shape domain-inverted inclusions in single crystal piezoelectric Z-cut lithium niobate. The band gaps appear at a frequency of about twice the Bragg band gap at the center of the Brillouin zone, formed through phonon-polariton coupling. The structure is mechanically, electromagnetically, and topographically homogeneous, without any physical alteration of the surface, offering an ideal platform for many acoustic wave applications for photonics, phononics, and microfluidics.
Phononic glass: a robust acoustic-absorption material.
Jiang, Heng; Wang, Yuren
2012-08-01
In order to achieve strong wide band acoustic absorption under high hydrostatic pressure, an interpenetrating network structure is introduced into the locally resonant phononic crystal to fabricate a type of phononic composite material called "phononic glass." Underwater acoustic absorption coefficient measurements show that the material owns high underwater sound absorption coefficients over 0.9 in 12-30 kHz. Moreover, the quasi-static compressive behavior shows that the phononic glass has a compressive strength over 5 MPa which is crucial for underwater applications.
NASA Astrophysics Data System (ADS)
Derov, John S.
1987-05-01
The literature was surveyed to determine potential applications of acoustic and plasma phenomena in superlattices. The use of folded zone acoustic phonons and acoustic surface plasmons in 3 to 5 compounds like AlGaAs/GaAs superlattices is addressed. A dielectric phonon filter is presented and an acoustic resonator is considered. Surface plasmons and surface acoustic plasmons are discussed and a transducer, delay line and mixer are proposed as applications. A 500 GHz isolator utilizing surface magnetoplasmons is also presented.
Single Circuit Parallel Computing with Phonons through Magneto-acoustics
NASA Astrophysics Data System (ADS)
Sklan, Sophia; Grossman, Jeffrey
2013-03-01
Phononic computing - the use of (typically thermal) vibrations for information processing - is a nascent technology; its capabilities are still being discovered. We analyze an alternative form of phononic computing inspired by optical, rather than electronic, computing. Using the acoustic Faraday effect, we design a phonon gyrator and thereby a means of performing computation through the manipulation of polarization in transverse phonon currents. Moreover, we establish that our gyrators act as generalized transistors and can construct digital logic gates. Exploiting the wave nature of phonons and the similarity of our logic gates, we demonstrate parallel computation within a single circuit, an effect presently unique to phonons. Finally, a generic method of designing these parallel circuits is introduced and used to analyze the feasibility of magneto-acoustic materials in realizing these circuits. This material is based upon work supported by the National Science Foundation Graduate Research Fellowship under Grant No. 1122374.
Acoustic phonon spectrum and thermal transport in nanoporous alumina arrays
Kargar, Fariborz; Ramirez, Sylvester; Debnath, Bishwajit; ...
2015-10-28
We report results of a combined investigation of thermal conductivity and acoustic phonon spectra in nanoporous alumina membranes with the pore diameter decreasing from D=180 nm to 25 nm. The samples with the hexagonally arranged pores were selected to have the same porosity Ø ≈13%. The Brillouin-Mandelstam spectroscopy measurements revealed bulk-like phonon spectrum in the samples with D = 180 nm pores and spectral features, which were attributed to spatial confinement, in the samples with 25 nm and 40 nm pores. The velocity of the longitudinal acoustic phonons was reduced in the samples with smaller pores. As a result, analysismore » of the experimental data and calculated phonon dispersion suggests that both phonon-boundary scattering and phonon spatial confinement affect heat conduction in membranes with the feature sizes D < 40 nm.« less
Acoustic phonon spectrum and thermal transport in nanoporous alumina arrays
Kargar, Fariborz; Ramirez, Sylvester; Debnath, Bishwajit; Malekpour, Hoda; Lake, Roger; Balandin, Alexander A.
2015-10-28
We report results of a combined investigation of thermal conductivity and acoustic phonon spectra in nanoporous alumina membranes with the pore diameter decreasing from D=180 nm to 25 nm. The samples with the hexagonally arranged pores were selected to have the same porosity Ø ≈13%. The Brillouin-Mandelstam spectroscopy measurements revealed bulk-like phonon spectrum in the samples with D = 180 nm pores and spectral features, which were attributed to spatial confinement, in the samples with 25 nm and 40 nm pores. The velocity of the longitudinal acoustic phonons was reduced in the samples with smaller pores. As a result, analysis of the experimental data and calculated phonon dispersion suggests that both phonon-boundary scattering and phonon spatial confinement affect heat conduction in membranes with the feature sizes D < 40 nm.
Acoustic Bloch oscillations in a two-dimensional phononic crystal
NASA Astrophysics Data System (ADS)
He, Zhaojian; Peng, Shasha; Cai, Feiyan; Ke, Manzhu; Liu, Zhengyou
2007-11-01
We report the observation of acoustic Bloch oscillations at megahertz frequency in a two-dimensional phononic crystal. By creating periodically arrayed cavities with a decreasing gradient in width along one direction in the phononic crystal, acoustic Wannier-Stark ladders are created in the frequency domain. The oscillatory motion of an incident Gaussian pulse inside the sample is demonstrated by both simulation and experiment.
The phononic crystals: An unending quest for tailoring acoustics
NASA Astrophysics Data System (ADS)
Kushwaha, Manvir S.
2016-07-01
Periodicity (in time or space) is a part and parcel of every living being: one can see, hear and feel it. Everyday examples are locomotion, respiration and heart beat. The reinforced N-dimensional periodicity over two or more crystalline solids results in the so-called phononic band gap crystals. These can have dramatic consequences on the propagation of phonons, vibrations and sound. The fundamental physics of cleverly fabricated phononic crystals can offer a systematic route to realize the Anderson localization of sound and vibrations. As to the applications, the phononic crystals are envisaged to find ways in the architecture, acoustic waveguides, designing transducers, elastic/acoustic filters, noise control, ultrasonics, medical imaging and acoustic cloaking, to mention a few. This review focuses on the brief sketch of the progress made in the field that seems to have prospered even more than was originally imagined in the early nineties.
Probing confined acoustic phonons in free standing small gold nanoparticles
Mankad, Venu; Jha, Prafulla K.; Ravindran, T. R.
2013-02-21
Polarized and depolarized spectra from gold (Au) nanoparticles of different sizes are investigated in the small size range, between 3 and 7 nm, using low frequency Raman spectroscopy. Acoustic vibrations of the free-standing Au nanoparticles are demonstrated with frequencies ranging from 5 to 35 cm{sup -1}, opening the way to the development of the acoustic resonators. A blue shift in the phonon peaks along with the broadening is observed with a decrease in particle size. Comparison of the measured frequencies with vibrational dynamics calculation and an examination as from the transmission electron microscopy results ascertain that the low frequency phonon modes are due to acoustic phonon quantization. Our results show that the observed low frequency Raman scattering originates from the spherical (l = 0) and quadrupolar (l = 2) vibrations of the spheroidal mode due to plasmon mediated acoustic vibrations in Au nanoparticles.
Stimulated emission of phonons in an acoustic cavity
NASA Astrophysics Data System (ADS)
Tilstra, Lieuwe Gijsbert
2001-10-01
This thesis will present experiments on stimulated emission of phonons in dilute ruby following complete population inversion of the Zeeman-split E(2E) Kramers doublet by selective pulsed optical pumping into its upper component. The resulting phonon avalanches are detected by use of the R1 luminescence emanating from the inverted zone, located near the end face where the laser beam enters the crystal. The phonons appear to team up into a highly directional phonon beam. The phonon frequency is tunable from, say, 10-100 GHz via the magnetic field splitting of the doublet. Remarkably, the population of the lower doublet component, which is a measure of the number of phonons generated, evolves with a sequence of distinct steps. The time interval in between these steps equals 2L/v, corresponding to the time the phonons need to return to the inverted zone by reflection at the opposite end face at a distance L. The end faces of the ruby crystal thus form an acoustic cavity. The phonon beam passes the inverted zone repeatedly to be amplified further, in a manner similar to light in an optical laser. In other words, the basic ingredients for a phonon laser have been established.
Slow light and slow acoustic phonons in optophononic resonators
NASA Astrophysics Data System (ADS)
Villafañe, V.; Soubelet, P.; Bruchhausen, A. E.; Lanzillotti-Kimura, N. D.; Jusserand, B.; Lemaître, A.; Fainstein, A.
2016-11-01
Slow and confined light have been exploited in optoelectronics to enhance light-matter interactions. Here we describe the GaAs/AlAs semiconductor microcavity as a device that, depending on the excitation conditions, either confines or slows down both light and optically generated acoustic phonons. The localization of photons and phonons in the same place of space amplifies optomechanical processes. Picosecond laser pulses are used to study through time-resolved reflectivity experiments the coupling between photons and both confined and slow acoustic phonons when the laser is tuned either with the cavity (confined) optical mode or with the stop-band edge (slow) optical modes. A model that fully takes into account the modified propagation of the acoustic phonons and light in these resonant structures is used to describe the laser detuning dependence of the coherently generated phonon spectra and amplitude under these different modes of laser excitation. We observe that confined light couples only to confined mechanical vibrations, while slow light can generate both confined and slow coherent vibrations. A strong enhancement of the optomechanical coupling using confined photons and vibrations, and also with properly designed slow photon and phonon modes, is demonstrated. The prospects for the use of these optoelectronic devices in confined and slow optomechanics are addressed.
Phononic crystal structures for acoustically driven microfluidic manipulations.
Wilson, Rab; Reboud, Julien; Bourquin, Yannyk; Neale, Steven L; Zhang, Yi; Cooper, Jonathan M
2011-01-21
The development of microfluidic systems is often constrained both by difficulties associated with the chip interconnection to other instruments and by limitations imposed by the mechanisms that can enable fluid movement and processing. Surface acoustic wave (SAW) devices have shown promise in allowing samples to be manipulated, although designing complex fluid operations involves using multiple electrode transducers. We now demonstrate a simple interface between a piezoelectric SAW device and a disposable microfluidic chip, patterned with phononic structures to control the acoustic wave propagation. The surface wave is coupled from the piezoelectric substrate into the disposable chip where it interacts with the phononic lattice. By implementing both a phononic filter and an acoustic waveguide, we illustrate the potential of the technique by demonstrating microcentrifugation for particle and cell concentration in microlitre droplets. We show for the first time that the interaction of the fluid within this metamaterial phononic lattice is dependent upon the frequency of the acoustic wave, providing a route to programme complex fluidic functions into a microchip (in much the same way, by analogy, that a holographic element would change the phase of a light wave in optical tweezers). A practical realisation of this involves the centrifugation of blood on the chip.
Nonlinear Transport and Noise Properties of Acoustic Phonons
NASA Astrophysics Data System (ADS)
Walczak, Kamil
We examine heat transport carried by acoustic phonons in molecular junctions composed of organic molecules coupled to two thermal baths of different temperatures. The phononic heat flux and its dynamical noise properties are analyzed within the scattering (Landauer) formalism with transmission probability function for acoustic phonons calculated within the method of atomistic Green's functions (AGF technique). The perturbative computational scheme is used to determine nonlinear corrections to phononic heat flux and its noise power spectral density with up to the second order terms with respect to temperature difference. Our results show the limited applicability of ballistic Fourier's law and fluctuation-dissipation theorem to heat transport in quantum systems. We also derive several noise-signal relations applicable to nanoscale heat flow carried by phonons, but valid for electrons as well. We also discuss the extension of the perturbative transport theory to higher order terms in order to address a huge variety of problems related to nonlinear thermal effects which may occur at nanoscale and at strongly non-equilibrium conditions with high-intensity heat fluxes. This work was supported by Pace University Start-up Grant.
Acoustic phonon transmission spectra in piezoelectric AlN/GaN Fibonacci phononic crystals
NASA Astrophysics Data System (ADS)
Sesion, P. D., Jr.; Albuquerque, E. L.; Chesman, C.; Freire, V. N.
2007-08-01
We study the acoustic-phonon transmission spectra in periodic and quasiperiodic (Fibonacci type) superlattices made up from the III-V nitride materials AlN and GaN. The phonon dynamics is described by a coupled elastic and electromagnetic equations within the static field approximation model, stressing the importance of the piezoelectric polarization field in a strained condition. We use a transfer-matrix treatment to simplify the algebra, which would be otherwise quite complicated, allowing a neat analytical expressions for the phonon transmission coefficients. Numerical results, for the normal incidence case, show a strike self-similar pattern for both hexagonal (class 6 mm) and cubic symmetries crystalizations of the nitrides.
Temperature Dependence of Brillouin Light Scattering Spectra of Acoustic Phonons in Silicon
NASA Astrophysics Data System (ADS)
Somerville, Kevin; Klimovich, Nikita; An, Kyongmo; Sullivan, Sean; Weathers, Annie; Shi, Li; Li, Xiaoqin
2015-03-01
Thermal management represents an outstanding challenge in many areas of technology. Electrons, optical phonons, and acoustic phonons are often driven out of local equilibrium in electronic devices or during laser-material interaction processes. Interest in non-equilibrium transport processes has motivated the development of Raman spectroscopy as a local temperature sensor of optical phonons and intermediate frequency acoustic phonons, whereas Brillouin light scattering (BLS) has recently been explored as a temperature sensor of low-frequency acoustic phonons. Here, we report temperature dependent BLS spectra of silicon, with Raman spectra taken simultaneously for comparison. The origins of the observed temperature dependence of the BLS peak position, linewidth, and intensity are examined in order to evaluate their potential use as temperature sensors for acoustic phonons. We determine that the integrated BLS intensity can be used measure the temperature of specific acoustic phonon modes. This work is supported by National Science Foundation (NSF) Thermal Transport Processes Program under Grant CBET-1336968.
Acoustic waves switch based on meta-fluid phononic crystals
NASA Astrophysics Data System (ADS)
Zhu, Xue-Feng
2012-08-01
The acoustic waves switch based on meta-fluid phononic crystals (MEFL PCs) is theoretically investigated. The MEFL PCs consist of fluid matrix and fluid-like inclusions with extremely anisotropic-density. The dispersion relations are calculated via the plane wave expansion method, which are in good agreement with the transmitted sound pressure level spectra obtained by the finite element method. The results show that the width of absolute band gap in MEFL PCs depends sensitively upon the orientation of the extremely anisotropic-density inclusions and reaches maximum at the rotating angle of 45°, with the gap position nearly unchanged. Also, the inter-mode conversion inside anisotropic-density inclusions can be ignored due to large acoustic mismatch. The study gives a possibility to realize greater flexibility and stronger effects in tuning the acoustic band gaps, which is very significant in the enhanced control over sound waves and has potential applications in ultrasonic imaging and therapy.
Magnetophonon oscillations caused by acoustic phonons in bulk conductors
NASA Astrophysics Data System (ADS)
Raichev, O. E.
2016-09-01
The interaction of electrons with acoustic phonons under a magnetic field leads to a remarkable kind of magnetophonon oscillation of transport coefficients, recently discovered in two-dimensional electron systems. The present study shows that similar oscillations exist in bulk conductors and provides a theory of this phenomenon for the case of spherical Fermi surfaces. The resonance peaks occur when the product of the Fermi surface diameter by the sound velocity is a multiple of the cyclotron frequency. Theoretical predictions may facilitate the experimental observation of the phenomenon.
Numerical investigation of diffraction of acoustic waves by phononic crystals
NASA Astrophysics Data System (ADS)
Moiseyenko, Rayisa P.; Declercq, Nico F.; Laude, Vincent
2012-05-01
Diffraction as well as transmission of acoustic waves by two-dimensional phononic crystals (PCs) composed of steel rods in water are investigated in this paper. The finite element simulations were performed in order to compute pressure fields generated by a line source that are incident on a finite size PC. Such field maps are analyzed based on the complex band structure for the infinite periodic PC. Finite size computations indicate that the exponential decrease of the transmission at deaf frequencies is much stronger than that in Bragg band gaps.
Temperature dependence of Brillouin light scattering spectra of acoustic phonons in silicon
Olsson, Kevin S.; Klimovich, Nikita; An, Kyongmo; Sullivan, Sean; Weathers, Annie; Shi, Li E-mail: elaineli@physics.utexas.edu; Li, Xiaoqin E-mail: elaineli@physics.utexas.edu
2015-02-02
Electrons, optical phonons, and acoustic phonons are often driven out of local equilibrium in electronic devices or during laser-material interaction processes. The need for a better understanding of such non-equilibrium transport processes has motivated the development of Raman spectroscopy as a local temperature sensor of optical phonons and intermediate frequency acoustic phonons, whereas Brillouin light scattering (BLS) has recently been explored as a temperature sensor of low-frequency acoustic phonons. Here, we report the measured BLS spectra of silicon at different temperatures. The origins of the observed temperature dependence of the BLS peak position, linewidth, and intensity are examined in order to evaluate their potential use as temperature sensors for acoustic phonons.
Temperature dependence of Brillouin light scattering spectra of acoustic phonons in silicon
NASA Astrophysics Data System (ADS)
Olsson, Kevin S.; Klimovich, Nikita; An, Kyongmo; Sullivan, Sean; Weathers, Annie; Shi, Li; Li, Xiaoqin
2015-02-01
Electrons, optical phonons, and acoustic phonons are often driven out of local equilibrium in electronic devices or during laser-material interaction processes. The need for a better understanding of such non-equilibrium transport processes has motivated the development of Raman spectroscopy as a local temperature sensor of optical phonons and intermediate frequency acoustic phonons, whereas Brillouin light scattering (BLS) has recently been explored as a temperature sensor of low-frequency acoustic phonons. Here, we report the measured BLS spectra of silicon at different temperatures. The origins of the observed temperature dependence of the BLS peak position, linewidth, and intensity are examined in order to evaluate their potential use as temperature sensors for acoustic phonons.
Effect of electron heating on femtosecond laser-induced coherent acoustic phonons in noble metals
NASA Astrophysics Data System (ADS)
Wang, Jincheng; Guo, Chunlei
2007-05-01
We employ a surface plasmon technique to resolve the dynamics of femtosecond-laser-induced coherent acoustic phonons in noble metals. Clear acoustic oscillations are observed in our experiments. We further study the dependence of the initial phase of the oscillations on pump fluence, and we find that the initial phase decreases linearly with pump fluence. Our model calculations show that hot electrons instantaneously excited by femtosecond pulses contribute to the generation of coherent acoustic phonons in metals.
Piezoelectric surface acoustical phonon amplification in graphene on a GaAs substrate
Nunes, O. A. C.
2014-06-21
We study the interaction of Dirac Fermions in monolayer graphene on a GaAs substrate in an applied electric field by the combined action of the extrinsic potential of piezoelectric surface acoustical phonons of GaAs (piezoelectric acoustical (PA)) and of the intrinsic deformation potential of acoustical phonons in graphene (deformation acoustical (DA)). We find that provided the dc field exceeds a threshold value, emission of piezoelectric (PA) and deformation (DA) acoustical phonons can be obtained in a wide frequency range up to terahertz at low and high temperatures. We found that the phonon amplification rate R{sup PA,DA} scales with T{sub BG}{sup S−1} (S=PA,DA), T{sub BG}{sup S} being the Block−Gru{sup ¨}neisen temperature. In the high-T Block−Gru{sup ¨}neisen regime, extrinsic PA phonon scattering is suppressed by intrinsic DA phonon scattering, where the ratio R{sup PA}/R{sup DA} scales with ≈1/√(n), n being the carrier concentration. We found that only for carrier concentration n≤10{sup 10}cm{sup −2}, R{sup PA}/R{sup DA}>1. In the low-T Block−Gru{sup ¨}neisen regime, and for n=10{sup 10}cm{sup −2}, the ratio R{sup PA}/R{sup DA} scales with T{sub BG}{sup DA}/T{sub BG}{sup PA}≈7.5 and R{sup PA}/R{sup DA}>1. In this regime, PA phonon dominates the electron scattering and R{sup PA}/R{sup DA}<1 otherwise. This study is relevant to the exploration of the acoustic properties of graphene and to the application of graphene as an acoustical phonon amplifier and a frequency-tunable acoustical phonon device.
Influence of confined acoustic phonons on the Radioelectric field in a Quantum well
NASA Astrophysics Data System (ADS)
Long, Do Tuan; Quang Bau, Nguyen
2015-06-01
The influence of confined acoustic phonons on the Radioelectric field in a quantum well has been studied in the presence of a linearly polarized electromagnetic wave and a laser radiation. By using the quantum kinetic equation for electrons with confined electrons - confined acoustic phonons interaction, the analytical expression for the Radio electric field is obtained. The formula of the Radio electric field contains the quantum number m characterizing the phonons confinement and comes back to the case of unconfined phonons when m reaches to zero. The dependence of the Radio electric field on the frequency of the laser radiation, in case of confined acoustic phonons, is also achieved by numerical method for a specific quantum well AlGaAs/GaAs/AlGaAs. Results show that the Radio electric field has a peak and reaches saturation as the frequency of the laser radiation increases.
NASA Astrophysics Data System (ADS)
Song, Ai-Ling; Chen, Tian-Ning; Wang, Xiao-Peng; Wan, Le-Le
2016-08-01
The waveform distortion happens in most of the unidirectional acoustic transmission (UAT) devices proposed before. In this paper, a novel type of waveform-preserved UAT device composed of an impedance-matched acoustic metasurface (AMS) and a phononic crystal (PC) structure is proposed and numerically investigated. The acoustic pressure field distributions and transmittance are calculated by using the finite element method. The subwavelength AMS that can modulate the wavefront of the transmitted wave at will is designed and the band structure of the PC structure is calculated and analyzed. The sound pressure field distributions demonstrate that the unidirectional acoustic transmission can be realized by the proposed UAT device without changing the waveforms of the output waves, which is the distinctive feature compared with the previous UAT devices. The physical mechanism of the unidirectional acoustic transmission is discussed by analyzing the refraction angle changes and partial band gap map. The calculated transmission spectra show that the UAT device is valid within a relatively broad frequency range. The simulation results agree well with the theoretical predictions. The proposed UAT device provides a good reference for designing waveform-preserved UAT devices and has potential applications in many fields, such as medical ultrasound, acoustic rectifiers, and noise insulation.
Kargar, Fariborz; Debnath, Bishwajit; Kakko, Joona-Pekko; Säynätjoki, Antti; Lipsanen, Harri; Nika, Denis L.; Lake, Roger K.; Balandin, Alexander A.
2016-01-01
Similar to electron waves, the phonon states in semiconductors can undergo changes induced by external boundaries. However, despite strong scientific and practical importance, conclusive experimental evidence of confined acoustic phonon polarization branches in individual free-standing nanostructures is lacking. Here we report results of Brillouin—Mandelstam light scattering spectroscopy, which reveal multiple (up to ten) confined acoustic phonon polarization branches in GaAs nanowires with a diameter as large as 128 nm, at a length scale that exceeds the grey phonon mean-free path in this material by almost an order-of-magnitude. The dispersion modification and energy scaling with diameter in individual nanowires are in excellent agreement with theory. The phonon confinement effects result in a decrease in the phonon group velocity along the nanowire axis and changes in the phonon density of states. The obtained results can lead to more efficient nanoscale control of acoustic phonons, with benefits for nanoelectronic, thermoelectric and spintronic devices. PMID:27830698
Propagation and localization of acoustic waves in Fibonacci phononic circuits
NASA Astrophysics Data System (ADS)
Aynaou, H.; El Boudouti, E. H.; Djafari-Rouhani, B.; Akjouj, A.; Velasco, V. R.
2005-07-01
A theoretical investigation is made of acoustic wave propagation in one-dimensional phononic bandgap structures made of slender tube loops pasted together with slender tubes of finite length according to a Fibonacci sequence. The band structure and transmission spectrum is studied for two particular cases. (i) Symmetric loop structures, which are shown to be equivalent to diameter-modulated slender tubes. In this case, it is found that besides the existence of extended and forbidden modes, some narrow frequency bands appear in the transmission spectra inside the gaps as defect modes. The spatial localization of the modes lying in the middle of the bands and at their edges is examined by means of the local density of states. The dependence of the bandgap structure on the slender tube diameters is presented. An analysis of the transmission phase time enables us to derive the group velocity as well as the density of states in these structures. In particular, the stop bands (localized modes) may give rise to unusual (strong normal) dispersion in the gaps, yielding fast (slow) group velocities above (below) the speed of sound. (ii) Asymmetric tube loop structures, where the loops play the role of resonators that may introduce transmission zeros and hence new gaps unnoticed in the case of simple diameter-modulated slender tubes. The Fibonacci scaling property has been checked for both cases (i) and (ii), and it holds for a periodicity of three or six depending on the nature of the substrates surrounding the structure.
Interface nano-confined acoustic waves in polymeric surface phononic crystals
Travagliati, Marco; Nardi, Damiano; Giannetti, Claudio; Ferrini, Gabriele; Banfi, Francesco; Gusev, Vitalyi; Pingue, Pasqualantonio; Piazza, Vincenzo
2015-01-12
The impulsive acoustic dynamics of soft polymeric surface phononic crystals is investigated here in the hypersonic frequency range by near-IR time-resolved optical diffraction. The acoustic response is analysed by means of wavelet spectral methods and finite element modeling. An unprecedented class of acoustic modes propagating within the polymer surface phononic crystal and confined within 100 nm of the nano-patterned interface is revealed. The present finding opens the path to an alternative paradigm for characterizing the mechanical properties of soft polymers at interfaces and for sensing schemes exploiting polymers as embedding materials.
Interface nano-confined acoustic waves in polymeric surface phononic crystals
NASA Astrophysics Data System (ADS)
Travagliati, Marco; Nardi, Damiano; Giannetti, Claudio; Gusev, Vitalyi; Pingue, Pasqualantonio; Piazza, Vincenzo; Ferrini, Gabriele; Banfi, Francesco
2015-01-01
The impulsive acoustic dynamics of soft polymeric surface phononic crystals is investigated here in the hypersonic frequency range by near-IR time-resolved optical diffraction. The acoustic response is analysed by means of wavelet spectral methods and finite element modeling. An unprecedented class of acoustic modes propagating within the polymer surface phononic crystal and confined within 100 nm of the nano-patterned interface is revealed. The present finding opens the path to an alternative paradigm for characterizing the mechanical properties of soft polymers at interfaces and for sensing schemes exploiting polymers as embedding materials.
Bleustein-Gulyaev-Shimizu surface acoustic waves in two-dimensional piezoelectric phononic crystals.
Hsu, Jin-Chen; Wu, Tsung-Tsong
2006-06-01
In this paper, we present a study on the existence of Bleustein-Gulyaev-Shimizu piezoelectric surface acoustic waves in a two-dimensional piezoelectric phononic crystal (zinc oxide, ZnO, and cadmium-sulfide, CdS) using the plane wave expansion method. In the configuration of ZnO (100)/CdS(100) phononic crystal, the calculated results show that this type of surface waves has higher acoustic wave velocities, high electromechanical coupling coefficients, and larger band gap width than those of the Rayleigh surface waves and pseudosurface waves. In addition, we find that the folded modes of the Bleustein-Gulyaev-Shimizu surface waves have higher coupling coefficients.
Mante, Pierre-Adrien; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.; Yartsev, Arkady
2017-01-01
Despite the great amount of attention CH3NH3PbI3 has received for its solar cell application, intrinsic properties of this material are still largely unknown. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. We apply this method to characterize a CH3NH3PbI3 single crystal. We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using the deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. Our results reveal high electron and hole mobilities of 2,800 and 9,400 cm2 V−1 s−1, respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3. PMID:28176755
Mante, Pierre-Adrien; Stoumpos, Constantinos C; Kanatzidis, Mercouri G; Yartsev, Arkady
2017-02-08
Despite the great amount of attention CH3NH3PbI3 has received for its solar cell application, intrinsic properties of this material are still largely unknown. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. We apply this method to characterize a CH3NH3PbI3 single crystal. We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using the deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. Our results reveal high electron and hole mobilities of 2,800 and 9,400 cm(2) V(-1) s(-1), respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3.
Mante, Pierre-Adrien; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.; ...
2017-02-08
The intrinsic properties of CH3NH3PbI3 are still largely unknown in spite of the great amount of attention it has received for its solar cell application. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. Furthermore, we apply this method to characterize a CH3NH3PbI3 single crystal.We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using themore » deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. These results reveal high electron and hole mobilities of 2,800 and 9,400 cm2V-1 s -1 , respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3.« less
NASA Astrophysics Data System (ADS)
Mante, Pierre-Adrien; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.; Yartsev, Arkady
2017-02-01
Despite the great amount of attention CH3NH3PbI3 has received for its solar cell application, intrinsic properties of this material are still largely unknown. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. We apply this method to characterize a CH3NH3PbI3 single crystal. We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using the deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. Our results reveal high electron and hole mobilities of 2,800 and 9,400 cm2 V-1 s-1, respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3.
Acoustic beam splitting at low GHz frequencies in a defect-free phononic crystal
NASA Astrophysics Data System (ADS)
Guo, Yuning; Brick, Delia; Großmann, Martin; Hettich, Mike; Dekorsy, Thomas
2017-01-01
The directional waveguiding in a 2D phononic crystal is simulated based on the analysis of equifrequency contours. This approach is utilized to investigate acoustic beam splitting in a defect-free nanostructure in the low GHz range. We find relaxed limitations regarding the source parameters compared to similar approaches in the sonic regime. Finally, we discuss the possibility to design an acoustic interferometer device at the nanoscale at GHz frequencies.
Acoustic phonon dynamics in thin-films of the topological insulator Bi2Se3
NASA Astrophysics Data System (ADS)
Glinka, Yuri D.; Babakiray, Sercan; Johnson, Trent A.; Holcomb, Mikel B.; Lederman, David
2015-04-01
Transient reflectivity traces measured for nanometer-sized films (6-40 nm) of the topological insulator Bi2Se3 revealed GHz-range oscillations driven within the relaxation of hot carriers photoexcited with ultrashort (˜100 fs) laser pulses of 1.51 eV photon energy. These oscillations have been suggested to result from acoustic phonon dynamics, including coherent longitudinal acoustic phonons in the form of standing acoustic waves. An increase of oscillation frequency from ˜35 to ˜70 GHz with decreasing film thickness from 40 to 15 nm was attributed to the interplay between two different regimes employing traveling-acoustic-waves for films thicker than 40 nm and the film bulk acoustic wave resonator (FBAWR) modes for films thinner than 40 nm. The amplitude of oscillations decays rapidly for films below 15 nm thick when the indirect intersurface coupling in Bi2Se3 films switches the FBAWR regime to that of the Lamb wave excitation. The frequency range of coherent longitudinal acoustic phonons is in good agreement with elastic properties of Bi2Se3.
Dexterous acoustic trapping and patterning of particles assisted by phononic crystal plate
Wang, Tian; Ke, Manzhu Xu, Shengjun; Feng, Junheng; Qiu, Chunyin; Liu, Zhengyou
2015-04-20
In this letter, we present experimental demonstration of multi-particles trapping and patterning by the artificially engineered acoustic field of phononic crystal plate. Polystyrene particles are precisely trapped and patterned in two dimensional arrays, for example, the square, triangular, or quasi-periodic arrays, depending on the structures of the phononic crystal plates with varying sub-wavelength holes array. Analysis shows that the enhanced acoustic radiation force, induced by the resonant transmission field highly localized near the sub-wavelength apertures, accounts for the particles self-organizing. It can be envisaged that this kind of simple design of phononic crystal plates would pave an alternative route for self-assembly of particles and may be utilized in the lab-on-a-chip devices.
Acoustic phonon dynamics in strained cubic and hexagonal GaN/Al2O3 superlattices
NASA Astrophysics Data System (ADS)
Sesion, P. D., Jr.; Albuquerque, E. L.; Vasconcelos, M. S.; Mauriz, P. W.; Freire, V. N.
2006-06-01
We study the acoustic-phonon spectra in periodic and quasiperiodic (Fibonacci type) superlattices made up from III V nitride materials (GaN) intercalated by sapphire (Al2O3). Due to the misalignments between the sapphire and the GaN layers that can lead to threading dislocation densities as high as 108-1010 cm-1, and a significant lattice mismatch (~14%), the phonon dynamics is described beyond the continuum elastic model using coupled elastic and electromagnetic equations, stressing the importance of the piezoelectric polarization field in a strained condition. We use a transfer-matrix treatment to simplify the algebra, which would be otherwise quite complicated, allowing a neat analytical expressions for the phonon dispersion relation. Furthermore, a quantitative analysis of the localization and magnitude of the allowed band widths in the phonon's spectra, as well as their scale law and the parametric spectrum of singularities f(α), are presented and discussed.
Observation of induced longitudinal and shear acoustic phonons by Brillouin scattering.
Yoshida, Taisuke; Matsukawa, Mami; Yanagitani, Takahiko
2011-06-01
To improve the accuracy of velocity measurements in the Brillouin scattering technique using weak thermal phonons, we have used induced coherent phonons, which intensify the scattering. To induce phonons in the gigahertz range, we used a c-axis tilted ZnO film transducer that was developed in our laboratory. This allowed us to induce longitudinal and shear acoustic phonons effectively at hypersonic frequencies. As a result, we obtained scattered light in the silica glass sample that was much more intense than that obtained from the thermal phonons. Because the Brillouin scattering from induced phonons was measured, the shift frequency was that of the electric signal applied to the ZnO transducer. Strong peaks lead to a reduction of the measurement time. This is useful for two-dimensional mapping of thin film elasticity using Brillouin scattering. Additionally, Brillouin scattering enables the simultaneous measurement of longitudinal and shear phonon velocities in the sample plane. This opens up a potential new technique for non-destructive elasticity measurements of various materials.
Design of acoustic beam aperture modifier using gradient-index phononic crystals
NASA Astrophysics Data System (ADS)
Lin, Sz-Chin Steven; Tittmann, Bernhard R.; Huang, Tony Jun
2012-06-01
This article reports the design concept of a novel acoustic beam aperture modifier using butt-jointed gradient-index phononic crystals (GRIN PCs) consisting of steel cylinders embedded in a homogeneous epoxy background. By gradually tuning the period of a GRIN PC, the propagating direction of acoustic waves can be continuously bent to follow a sinusoidal trajectory in the structure. The aperture of an acoustic beam can therefore be shrunk or expanded through change of the gradient refractive index profiles of the butt-jointed GRIN PCs. Our computational results elucidate the effectiveness of the proposed acoustic beam aperture modifier. Such an acoustic device can be fabricated through a simple process and will be valuable in applications, such as biomedical imaging and surgery, nondestructive evaluation, communication, and acoustic absorbers.
Multi-resonance tunneling of acoustic waves in two-dimensional locally-resonant phononic crystals
NASA Astrophysics Data System (ADS)
Yang, Aichao; He, Wei; Zhang, Jitao; Zhu, Liang; Yu, Lingang; Ma, Jian; Zou, Yang; Li, Min; Wu, Yu
2017-03-01
Multi-resonance tunneling of acoustic waves through a two-dimensional phononic crystal (PC) is demonstrated by substituting dual Helmholtz resonators (DHRs) for acoustically-rigid scatterers in the PC. Due to the coupling of the incident waves with the acoustic multi-resonance modes of the DHRs, acoustic waves can tunnel through the PC at specific frequencies which lie inside the band gaps of the PC. This wave tunneling transmission can be further broadened by using the multilayer Helmholtz resonators. Thus, a PC consisting of an array of dual/multilayer Helmholtz resonators can serve as an acoustic band-pass filter, used to pick out acoustic waves with certain frequencies from noise.
Sub-Poissonian phonon statistics in an acoustical resonator coupled to a pumped two-level emitter
NASA Astrophysics Data System (ADS)
Ceban, V.; Macovei, M. A.
2015-11-01
The concept of an acoustical analog of the optical laser has been developed recently in both theoretical and experimental works. We here discuss a model of a coherent phonon generator with a direct signature of the quantum properties of sound vibrations. The considered setup is made of a laser-driven quantum dot embedded in an acoustical nanocavity. The system dynamics is solved for a single phonon mode in the steady-state and in the strong quantum dot—phonon coupling regime beyond the secular approximation. We demonstrate that the phonon statistics exhibits quantum features, i.e., is sub-Poissonian.
Sub-Poissonian phonon statistics in an acoustical resonator coupled to a pumped two-level emitter
Ceban, V. Macovei, M. A.
2015-11-15
The concept of an acoustical analog of the optical laser has been developed recently in both theoretical and experimental works. We here discuss a model of a coherent phonon generator with a direct signature of the quantum properties of sound vibrations. The considered setup is made of a laser-driven quantum dot embedded in an acoustical nanocavity. The system dynamics is solved for a single phonon mode in the steady-state and in the strong quantum dot—phonon coupling regime beyond the secular approximation. We demonstrate that the phonon statistics exhibits quantum features, i.e., is sub-Poissonian.
Peculiar transmission property of acoustic waves in a one-dimensional layered phononic crystal
NASA Astrophysics Data System (ADS)
Zhao, Degang; Wang, Wengang; Liu, Zhengyou; Shi, Jing; Wen, Weijia
2007-03-01
In this article, we report both theoretical calculation and experimental observation of acoustic waves abnormally through a one-dimensional layered transmitted phononic crystal at frequencies within the band gap into a material of large acoustic impedance mismatch, with an efficiency as high as unity. The transmission peaks can be interpreted as a result of the interference of acoustic waves reflected from all periodically aligned interfaces. The condition for the appearance of peaks is analyzed in detail and the optimized layer number is given for different configurations.
Role of acoustic phonons in frequency dependent electronic thermal conductivity of graphene
NASA Astrophysics Data System (ADS)
Bhalla, Pankaj
2017-03-01
We study the effect of the electron-phonon interaction on the finite frequency dependent electronic thermal conductivity of two dimensional graphene. We calculate it for various acoustic phonons present in graphene and characterized by different dispersion relations using the memory function approach. It is found that the electronic thermal conductivity κe (T) in the zero frequency limit follows different power law for the longitudinal/transverse and the flexural acoustic phonons. For the longitudinal/transverse phonons, κe (T) ∼T-1 at the low temperature and saturates at the high temperature. These signatures qualitatively agree with the results calculated by solving the Boltzmann equation analytically and numerically. Similarly, for the flexural phonons, we find that κe (T) shows T 1 / 2 law at the low temperature and then saturates at the high temperature. In the finite frequency regime, we observe that the real part of the electronic thermal conductivity, Re [κe (ω , T) ] follows ω-2 behavior at the low frequency and becomes frequency independent at the high frequency.
Acoustic phonon propagation in ultra-thin Si membranes under biaxial stress field
NASA Astrophysics Data System (ADS)
Graczykowski, B.; Gomis-Bresco, J.; Alzina, F.; Reparaz, J. S.; Shchepetov, A.; Prunnila, M.; Ahopelto, J.; Sotomayor Torres, C. M.
2014-07-01
We report on stress induced changes in the dispersion relations of acoustic phonons propagating in 27 nm thick single crystalline Si membranes. The static tensile stress (up to 0.3 GPa) acting on the Si membranes was achieved using an additional strain compensating silicon nitride frame. Dispersion relations of thermally activated hypersonic phonons were measured by means of Brillouin light scattering spectroscopy. The theory of Lamb wave propagation is developed for anisotropic materials subjected to an external static stress field. The dispersion relations were calculated using the elastic continuum approximation and taking into account the acousto-elastic effect. We find an excellent agreement between the theoretical and the experimental dispersion relations.
Decoupling of multiple coupled phononic crystal waveguides: application to acoustic demultiplexing
NASA Astrophysics Data System (ADS)
Zou, Qiushun; Liu, Wenxing; Yu, Tianbao; Liu, Nianhua; Wang, Tongbiao; Liao, Qinghua
2017-03-01
We show that the decoupling of two coupled phononic crystal waveguides (PnCWs) by a proper design can be achieved. And this decoupling property can be extended to the coupling of any number of parallel coupled PnCWs. The acoustic wavelength for decoupling is insensitive to the number of coupled PnCWs. Decoupling induces the extinction of neighbor PnCWs’ power transfer and makes the design of compact acoustic components easier. As a possible application of our work, a new kind of 1-to-2 acoustic demultiplexers are numerically demonstrated by employing the decoupling at the crossing-point frequency in two and three coupled PnCWs. This design concept provides a novel method and compact model for acoustic demultiplexing and can present practical applications in future acoustic wave circuits.
Persson, A. I. H.; Andreasson, B. P.; Enquist, H.; Jurgilaitis, A.; Larsson, J.
2015-11-14
The spectrum of laser-generated acoustic phonons in indium antimonide coated with a thin nickel film has been studied using time-resolved x-ray diffraction. Strain pulses that can be considered to be built up from coherent phonons were generated in the nickel film by absorption of short laser pulses. Acoustic reflections at the Ni–InSb interface leads to interference that strongly modifies the resulting phonon spectrum. The study was performed with high momentum transfer resolution together with high time resolution. This was achieved by using a third-generation synchrotron radiation source that provided a high-brightness beam and an ultrafast x-ray streak camera to obtain a temporal resolution of 10 ps. We also carried out simulations, using commercial finite element software packages and on-line dynamic diffraction tools. Using these tools, it is possible to calculate the time-resolved x-ray reflectivity from these complicated strain shapes. The acoustic pulses have a peak strain amplitude close to 1%, and we investigated the possibility to use this device as an x-ray switch. At a bright source optimized for hard x-ray generation, the low reflectivity may be an acceptable trade-off to obtain a pulse duration that is more than an order of magnitude shorter.
Long-Lived, Coherent Acoustic Phonon Oscillations in GaN Single Crystals
Wu, S.; Geiser, P.; Jun, J.; Karpinski, J.; Park, J.-R.; Sobolewski, R.
2006-01-31
We report on coherent acoustic phonon (CAP) oscillations studied in high-quality bulk GaN single crystals with a two-color femtosecond optical pump-probe technique. Using a far-above-the-band gap ultraviolet excitation (~270 nm wavelength) and a near-infrared probe beam (~810 nm wavelength), the long-lived, CAP transients were observed within a 10 ns time-delay window between the pump and probe pulses, with a dispersionless (proportional to the probe-beam wave vector) frequency of ~45 GHz. The measured CAP attenuation corresponded directly to the absorption of the probe light in bulk GaN, indicating that the actual (intrinsic) phonon-wave attenuation in our crystals was significantly smaller than the measured 65.8 cm^-1 value. The velocity of the phonon propagation was equal to the velocity of sound in GaN.
NASA Astrophysics Data System (ADS)
Srikanthreddy, D.; Glavin, B. A.; Poyser, C. L.; Henini, M.; Lehmann, D.; Jasiukiewicz, Cz.; Akimov, A. V.; Kent, A. J.
2017-02-01
We study the generation of microwave electronic signals by pumping a (311) GaAs Schottky diode with compressive and shear acoustic phonons, generated by the femtosecond optical excitation of an Al film transducer and mode conversion at the Al-GaAs interface. They propagate through the substrate and arrive at the Schottky device on the opposite surface, where they induce a microwave electronic signal. The arrival time, the amplitude, and the polarity of the signals depend on the phonon mode. A theoretical analysis is made of the polarity of the experimental signals. This analysis includes the piezoelectric and deformation potential mechanisms of electron-phonon interaction in a Schottky contact and shows that the piezoelectric mechanism is dominant for both transverse and longitudinal modes with frequencies below 250 and 70 GHz, respectively.
Acoustic beam splitting in two-dimensional phononic crystals using self-collimation effect
Li, Jing; Wu, Fugen Zhong, Huilin; Yao, Yuanwei; Zhang, Xin
2015-10-14
We propose two models of self-collimation-based beam splitters in phononic crystals. The finite element method is used to investigate the propagation properties of acoustic waves in two-dimensional phononic crystals. The calculated results show that the efficiency of the beam splitter can be controlled systematically by varying the radius of the rods or by changing the orientation of the square rods in the line defect. The effect of changing the side length of the square rods on acoustic wave propagation is discussed. The results show that the total transmission/reflection range decreases/increases as the side length increases. We also find that the relationship between the orientation of the transflective point and the side length of the square rods is quasi-linear.
Acoustic phonon lifetimes and thermal transport in free-standing and strained graphene.
Bonini, Nicola; Garg, Jivtesh; Marzari, Nicola
2012-06-13
We use first-principles methods based on density functional perturbation theory to characterize the lifetimes of the acoustic phonon modes and their consequences on the thermal transport properties of graphene. We show that using a standard perturbative approach, the transverse and longitudinal acoustic phonons in free-standing graphene display finite lifetimes in the long-wavelength limit, making them ill-defined as elementary excitations in samples of dimensions larger than ∼1 μm. This behavior is entirely due to the presence of the quadratic dispersions for the out-of-plane phonon (ZA) flexural modes that appear in free-standing low-dimensional systems. Mechanical strain lifts this anomaly, and all phonons remain well-defined at any wavelength. Thermal transport is dominated by ZA modes, and the thermal conductivity is predicted to diverge with system size for any amount of strain. These findings highlight strain and sample size as key parameters in characterizing or engineering heat transport in graphene.
Cooling phonons with phonons: Acoustic reservoir engineering with silicon-vacancy centers in diamond
NASA Astrophysics Data System (ADS)
Kepesidis, K. V.; Lemonde, M.-A.; Norambuena, A.; Maze, J. R.; Rabl, P.
2016-12-01
We study a setup where a single negatively-charged silicon-vacancy center in diamond is magnetically coupled to a low-frequency mechanical bending mode and via strain to the high-frequency phonon continuum of a semiclamped diamond beam. We show that under appropriate microwave driving conditions, this setup can be used to induce a laser-cooling-like effect for the low-frequency mechanical vibrations, where the high-frequency longitudinal compression modes of the beam serve as an intrinsic low-temperature reservoir. We evaluate the experimental conditions under which cooling close to the quantum ground state can be achieved and describe an extended scheme for the preparation of a stationary entangled state between two mechanical modes. By relying on intrinsic properties of the mechanical beam only, this approach offers an interesting alternative for quantum manipulation schemes of mechanical systems, where otherwise efficient optomechanical interactions are not available.
Demonstration of acoustic waveguiding and tight bending in phononic crystals
Ghasemi Baboly, M.; Raza, A.; Brady, J.; ...
2016-10-31
The systematic design, fabrication, and characterization of an isolated, single-mode, 90° bend phononic crystal (PnC) waveguide are presented. A PnC consisting of a 2D square array of circular air holes in an aluminum substrate is used, and waveguides are created by introducing a line defect in the PnC lattice. A high transmission coefficient is observed (–1 dB) for the straight sections of the waveguide, and an overall 2.3 dB transmission loss is observed (a transmission coefficient of 76%) for the 90° bend. Further optimization of the structure may yield higher transmission efficiencies. Lastly, this manuscript shows the complete design processmore » for an engineered 90° bend PnC waveguide from inception to experimental demonstration.« less
Demonstration of acoustic waveguiding and tight bending in phononic crystals
Ghasemi Baboly, M.; Raza, A.; Brady, J.; Reinke, C. M.; Leseman, Z. C.; El-Kady, I.
2016-10-31
The systematic design, fabrication, and characterization of an isolated, single-mode, 90° bend phononic crystal (PnC) waveguide are presented. A PnC consisting of a 2D square array of circular air holes in an aluminum substrate is used, and waveguides are created by introducing a line defect in the PnC lattice. A high transmission coefficient is observed (–1 dB) for the straight sections of the waveguide, and an overall 2.3 dB transmission loss is observed (a transmission coefficient of 76%) for the 90° bend. Further optimization of the structure may yield higher transmission efficiencies. Lastly, this manuscript shows the complete design process for an engineered 90° bend PnC waveguide from inception to experimental demonstration.
NASA Astrophysics Data System (ADS)
Kang, Hwi Suk; Yoon, Suk Wang; Lee, Kang Il
2017-02-01
In the present study, we experimentally and theoretically demonstrated anomalous negative reflection of acoustic waves obliquely incident upon the boundary of a two-dimensional phononic crystal (PC) consisting of periodic square arrays of stainless-steel cylinders immersed in water. The angular spectrogram showing the frequency as a function of the angle was measured for the reflection from the PC when the incidence angle of the sound beam was fixed to be 20°. To understand the negative reflection from the PC, we considered the boundary of the PC to behave as an acoustic diffraction grating, and we calculated the acoustic pressure fields at specific frequencies of interest by using the finite element method. We found that the grating law could be successfully applied to the boundary of the PC in order to determine the direction of the acoustic waves diffracted in water.
Intrinsic coherent acoustic phonons in the indirect band gap semiconductors Si and GaP
NASA Astrophysics Data System (ADS)
Ishioka, Kunie; Rustagi, Avinash; Höfer, Ulrich; Petek, Hrvoje; Stanton, Christopher J.
2017-01-01
We report on the intrinsic optical generation and detection of coherent acoustic phonons at (001)-oriented bulk Si and GaP without metallic phonon transducer structures. Photoexcitation by a 3.1-eV laser pulse generates a normal strain pulse within the ˜100 -nm penetration depth in both semiconductors. The subsequent propagation of the strain pulse into the bulk is detected with a delayed optical probe as a periodic modulation of the optical reflectivity. Our theoretical model explains quantitatively the generation of the acoustic pulse via the deformation potential electron-phonon coupling and detection in terms of the spatially and temporally dependent photoelastic effect for both semiconductors. Comparison with our theoretical model reveals that the experimental strain pulses have finite buildup times of 1.2 and 0.4 ps for GaP and Si, which are comparable with the time required for the photoexcited electrons to transfer to the lowest X valley through intervalley scattering. The deformation potential coupling related to the acoustic pulse generation for GaP is estimated to be twice as strong as that for Si from our experiments, in agreement with a previous theoretical prediction.
Graczykowski, B. Alzina, F.; Gomis-Bresco, J.; Sotomayor Torres, C. M.
2016-01-14
In this paper, we report a theoretical investigation of surface acoustic waves propagating in one-dimensional phononic crystal. Using finite element method eigenfrequency and frequency response studies, we develop two model geometries suitable to distinguish true and pseudo (or leaky) surface acoustic waves and determine their propagation through finite size phononic crystals, respectively. The novelty of the first model comes from the application of a surface-like criterion and, additionally, functional damping domain. Exemplary calculated band diagrams show sorted branches of true and pseudo surface acoustic waves and their quantified surface confinement. The second model gives a complementary study of transmission, reflection, and surface-to-bulk losses of Rayleigh surface waves in the case of a phononic crystal with a finite number of periods. Here, we demonstrate that a non-zero transmission within non-radiative band gaps can be carried via leaky modes originating from the coupling of local resonances with propagating waves in the substrate. Finally, we show that the transmission, reflection, and surface-to-bulk losses can be effectively optimised by tuning the geometrical properties of a stripe.
Wave propagation and acoustic band gaps of two-dimensional liquid crystal/solid phononic crystals
NASA Astrophysics Data System (ADS)
Oltulu, Oral; Mamedov, Amirullah M.; Ozbay, Ekmel
2017-01-01
The vast majority of acoustic wave propagation in phononic band studies has been usually carried out by scattering inclusions embedded in a viscoelastic medium, such as air or water. In this study, we present calculated band structure results for the two-dimensional square array geometry of a solid cylindrical scatterer surrounded by a liquid crystal (LC) matrix. Liquid crystals provide a unique combination of liquid-like and crystal-like properties as well as anisotropic properties. The purpose of using LC material is to take advantage of longitudinal acoustic waves propagating parallel (||) and perpendicular (⊥) to the nematic liquid crystal (NLC) director n. The compound used in this study was a room temperature NLC, called 5CB (4-pentyl-4'-cyanobiphenyl). The acoustic band structure of a two-dimensional phononic crystal containing a 5CB NLC and lithium tantalate was investigated by the plane wave expansion method. The theoretical results show that the solid/LC system can be tuned in a favorable configuration for adjusting or shifting acoustic band gaps.
Addouche, Mahmoud Al-Lethawe, Mohammed A. Choujaa, Abdelkrim Khelif, Abdelkrim
2014-07-14
We demonstrate super resolution imaging for surface acoustic waves using a phononic structure displaying negative refractive index. This phononic structure is made of a monolithic square lattice of cylindrical pillars standing on a semi-infinite medium. The pillars act as acoustic resonator and induce a surface propagating wave with unusual dispersion. We found, under specific geometrical parameters, one propagating mode that exhibits negative refraction effect with negative effective index close to −1. Furthermore, a flat lens with finite number of pillars is designed to allow the focusing of an acoustic point source into an image with a resolution of (λ)/3 , overcoming the Rayleigh diffraction limit.
Guiding and confinement of interface acoustic waves in solid-fluid pillar-based phononic crystals
NASA Astrophysics Data System (ADS)
Razip Wee, M. F. Mohd; Addouche, Mahmoud; Siow, Kim S.; Zain, A. R. Md; Elayouch, Aliyasin; Chollet, Franck; Khelif, Abdelkrim
2016-12-01
Pillar-based phononic crystals exhibit some unique wave phenomena due to the interaction between surface acoustic modes of the substrate and local resonances supported by pillars. In this paper, we extend the investigations by taking into account the presence of a liquid medium. We particularly demonstrate that local resonances dramatically decrease the phase velocity of Scholte-Stoneley wave, which leads to a slow wave at the solid/fluid interface. Moreover, we show that increasing the height of pillars introduces a new set of branches of interface modes and drastically affects the acoustic energy localization. Indeed, while some modes display a highly confined pressure between pillars, others exponentially decay in the fluid or only propagate in the solid without disturbing the fluid pressure. These theoretical results, performed by finite element method, highlight a new acoustic wave confinement suitable in various applications such as acoustophoresis, lab on chip and microfluidics.
2011-01-01
High-frequency surface acoustic waves can be generated by ultrafast laser excitation of nanoscale patterned surfaces. Here we study this phenomenon in the hypersonic frequency limit. By modeling the thermomechanics from first-principles, we calculate the system’s initial heat-driven impulsive response and follow its time evolution. A scheme is introduced to quantitatively access frequencies and lifetimes of the composite system’s excited eigenmodes. A spectral decomposition of the calculated response on the eigemodes of the system reveals asymmetric resonances that result from the coupling between surface and bulk acoustic modes. This finding allows evaluation of impulsively excited pseudosurface acoustic wave frequencies and lifetimes and expands our understanding of the scattering of surface waves in mesoscale metamaterials. The model is successfully benchmarked against time-resolved optical diffraction measurements performed on one-dimensional and two-dimensional surface phononic crystals, probed using light at extreme ultraviolet and near-infrared wavelengths. PMID:21910426
Acoustic phonons in chrysotile asbestos probed by high-resolution inelastic x-ray scattering
Mamontov, Eugene; Vakhrushev, S. B.; Kumzerov, Yu. A,; Alatas, A.
2009-01-01
Acoustic phonons in an individual, oriented fiber of chrysotile asbestos (chemical formula Mg{sub 3}Si{sub 2}O{sub 5}(OH){sub 4}) were observed at room temperature in the inelastic x-ray measurement with a very high (meV) resolution. The x-ray scattering vector was aligned along [1 0 0] direction of the reciprocal lattice, nearly parallel to the long axis of the fiber. The latter coincides with [1 0 0] direction of the direct lattice and the axes of the nano-channels. The data were analyzed using a damped harmonic oscillator model. Analysis of the phonon dispersion in the first Brillouin zone yielded the longitudinal sound velocity of (9200 {+-} 600) m/s.
Coherent longitudinal acoustic phonons in three-dimensional supracrystals of cobalt nanocrystals.
Lisiecki, Isabelle; Polli, Dario; Yan, Cong; Soavi, Giancarlo; Duval, Eugène; Cerullo, Giulio; Pileni, Marie-Paule
2013-10-09
We use broadband picosecond acoustics to detect longitudinal acoustic phonons with few-gigahertz frequency in three-dimensional supracrystals (with face-centered cubic lattice) of 7 nm cobalt nanocrystal spheres. In full analogy with atomic crystals, where longitudinal acoustic phonons propagate with the speed of sound through coherent movements of atoms of the lattice out of their equilibrium positions, in these supracrystals atoms are replaced by (uncompressible) nanocrystals and atomic bonds by coating agents (carbon chains) that act like mechanical springs holding together the nanocrystals. By repeating the measurements at different laser angles of incidence it was possible to accurately determine both the index of refraction of the supracrystal (n = 1.26 ± 0.03) and the room-temperature longitudinal speed of sound (v(s)= 1235 ± 12 m/s), which is quite low due to the heavy weight of the spheres (with respect to atoms in a crystal) and the soft carbon chains (with respect to atomic bonds). Interestingly, the speed of sound inside the supracrystal was found to dramatically increase by decreasing the sample temperature due to a change in the stiffness of the dodecanoic acid chains which coat the Co nanocrystals.
Pandya, Ankur; Shinde, Satyam; Jha, Prafulla K.
2015-05-15
In this paper the hot electron transport properties like carrier energy and momentum scattering rates and electron energy loss rates are calculated via interactions of electrons with polar acoustical phonons for Mn doped BN quantum well in BN nanosheets via piezoelectric scattering and deformation potential mechanisms at low temperatures with high electric field. Electron energy loss rate increases with the electric field. It is observed that at low temperatures and for low electric field the phonon absorption is taking place whereas, for sufficient large electric field, phonon emission takes place. Under the piezoelectric (polar acoustical phonon) scattering mechanism, the carrier scattering rate decreases with the reduction of electric field at low temperatures wherein, the scattering rate variation with electric field is limited by a specific temperature beyond which there is no any impact of electric field on such scattering.
Controlled exciton transfer between quantum dots with acoustic phonons taken into account
Golovinski, P. A.
2015-09-15
A system of excitons in two quantum dots coupled by the dipole–dipole interaction is investigated. The excitation transfer process controlled by the optical Stark effect at nonresonant frequencies is considered and the effect of the interaction between excitons and acoustic phonons in a medium on this process is taken into account. The system evolution is described using quantum Heisenberg equations. A truncated set of equations is obtained and the transfer dynamics is numerically simulated. High-efficiency picosecond switching of the excitation transfer by a laser pulse with a rectangular envelope is demonstrated. The dependence of picosecond switching on the quantum-dot parameters and optical-pulse length is presented.
Tunneling times of acoustic phonon packets through a distributed Bragg reflector
2014-01-01
The longwave phenomenological model is used to make simple and precise calculations of various physical quantities such as the vibrational energy density, the vibrational energy, the relative mechanical displacement, and the one-dimensional stress tensor of a porous silicon distributed Bragg reflector. From general principles such as invariance under time reversal, invariance under space reflection, and conservation of energy density flux, the equivalence of the tunneling times for both transmission and reflection is demonstrated. Here, we study the tunneling times of acoustic phonon packets through a distributed Bragg reflector in porous silicon multilayer structures, and we report the possibility that a phenomenon called Hartman effect appears in these structures. PMID:25237288
Coherent acoustic phonon generation in GaAs{sub 1−x}Bi{sub x}
Joshya, R. S.; Kini, R. N.; Ptak, A. J.; France, R.; Mascarenhas, A.
2014-03-03
We have used femtosecond laser pulses to generate coherent acoustic phonons in the dilute Bismide alloy, GaAs{sub 1−x}Bi{sub x}. The observed oscillation periods match well with the oscillation periods calculated using the propagating strain pulse model. We attribute the generation process predominantly to electronic stress due to the absorption of the laser pulse at the surface of the GaAs{sub 1−x}Bi{sub x} layer. Our initial estimates suggest that the incorporation of Bi in GaAs causes an enhancement of the hydrostatic deformation potential because of the resonant state in the valence band due to isolated Bi impurities.
Richardson, M.; Bhethanabotla, V. R.; Sankaranarayanan, S. K. R. S.
2014-06-23
Finite element simulations of a phononic shear-horizontal surface acoustic wave (SAW) sensor based on ST 90°-X Quartz reveal a dramatic reduction in power consumption. The phononic sensor is realized by artificially structuring the delay path to form an acoustic meta-material comprised of a periodic microcavity array incorporating high-density materials such as tantalum or tungsten. Constructive interference of the scattered and secondary reflected waves at every microcavity interface leads to acoustic energy confinement in the high-density regions translating into reduced power loss. Tantalum filled cavities show the best performance while tungsten inclusions create a phononic bandgap. Based on our simulation results, SAW devices with tantalum filled microcavities were fabricated and shown to significantly decrease insertion loss. Our findings offer encouraging prospects for designing low power, highly sensitive portable biosensors.
Continuum approach for long-wavelength acoustic phonons in quasi-two-dimensional structures
NASA Astrophysics Data System (ADS)
Liu, Dan; Every, Arthur G.; Tománek, David
2016-10-01
As an alternative to atomistic calculations of long-wavelength acoustic modes of atomically thin layers, which are known to converge very slowly, we propose a quantitatively predictive and physically intuitive approach based on continuum elasticity theory. We describe a layer, independent of its thickness, by a membrane and characterize its elastic behavior by a (3 ×3 ) elastic matrix as well as the flexural rigidity. We present simple quantitative expressions for frequencies of long-wavelength acoustic modes, which we determine using two-dimensional elastic constants calculated by ab initio density functional theory. The calculated spectra accurately reproduce observed and calculated long-wavelength phonon spectra of graphene and phosphorene, the monolayer of black phosphorus. Our approach also correctly describes the observed dependence of the radial breathing mode frequency on the diameters of carbon fullerenes and nanotubes.
Surface acoustic waves in two dimensional phononic crystal with anisotropic inclusions
NASA Astrophysics Data System (ADS)
Ketata, H.; Hédi Ben Ghozlen, M.
2012-06-01
An analysis is given to the band structure of the two dimensional solid phononic crystal considered as a semi infinite medium. The lattice includes an array of elastic anisotropic materials with different shapes embedded in a uniform matrix. For illustration two kinds of phononic materials are assumed. A particular attention is devoted to the computational procedure which is mainly based on the plane wave expansion (PWE) method. It has been adapted to Matlab environment. Numerical calculations of the dispersion curves have been achieved by introducing particular functions which transform motion equations into an Eigen value problem. Significant improvements are obtained by increasing reasonably the number of Fourier components even when a large elastic mismatch is assumed. Such approach can be generalized to different types of symmetry and permit new physical properties as piezoelectricity to be added. The actual semi infinite phononic structure with a free surface has been shown to support surface acoustic waves (SAW). The obtained dispersion curves reveal band gaps in the SAW branches. It has been found that the influence, of the filling factor and anisotropy on their band gaps, is different from that of bulk waves.
Morvan, B.; Tinel, A.; Sainidou, R.; Rembert, P.; Vasseur, J. O.; Hladky-Hennion, A.-C.; Swinteck, N.; Deymier, P. A.
2014-12-07
Phononic crystals (PC) can be used to control the dispersion properties of acoustic waves, which are essential to direct their propagation. We use a PC-based two-dimensional solid/solid composite to demonstrate experimentally and theoretically the spatial filtering of a monochromatic non-directional wave source and its emission in a surrounding water medium as an ultra-directional beam with narrow angular distribution. The phenomenon relies on square-shaped equifrequency contours (EFC) enabling self-collimation of acoustic waves within the phononic crystal. Additionally, the angular width of collimated beams is controlled via the EFC size-shrinking when increasing frequency.
NASA Astrophysics Data System (ADS)
Gao, Nansha; Wu, Jiu Hui; Yu, Lie; Hou, Hong
2016-06-01
This paper investigates ultralow frequency acoustic properties and energy recovery of tetragonal folding beam phononic crystal (TFBPC) and its complementary structure. The dispersion curve relationships, transmission spectra and displacement fields of the eigenmodes are studied with FEA in detail. Compared with the traditional three layer phononic crystal (PC) structure, this structure proposed in this paper not only unfold bandgaps (BGs) in lower frequency range (below 300 Hz), but also has lighter weight because of beam structural cracks. We analyze the relevant physical mechanism behind this phenomenon, and discuss the effects of the tetragonal folding beam geometric parameters on band structure maps. FEM proves that the multi-cell structures with different arrangements have different acoustic BGs when compared with single cell structure. Harmonic frequency response and piezoelectric properties of TFBPC are specifically analyzed. The results confirm that this structure does have the recovery ability for low frequency vibration energy in environment. These conclusions in this paper could be indispensable to PC practical applications such as BG tuning and could be applied in portable devices, wireless sensor, micro-electro mechanical systems which can recycle energy from vibration environment as its own energy supply.
NASA Astrophysics Data System (ADS)
Bhargavi, K. S.; Kubakaddi, S. S.
2016-09-01
The amplification coefficient α of acoustic phonons is theoretically investigated in a three-dimensional Dirac semimetal (3DDS) driven by a dc electric field E causing the drift of the electrons. It is numerically studied as a function of the frequency ωq, drift velocity vd, electron concentration ne, and temperature T in the Dirac semimetal Cd3As2. We find that the amplification of acoustic phonons (α ˜ hundreds of cm-1) takes place when the electron drift velocity vd is greater than the sound velocity vs. The amplification is found to occur at small E (˜few V/cm) due to large electron mobility. The frequency dependence of α shows amplification in the THz regime with a maximum αm occurring at the same frequency ωqm for different vd. The αm is found to increase with increasing vd. α vs ωq for different ne also shows a maximum, with αm shifting to higher ωq for larger ne. Each maximum is followed by a vanishing α at nearly "2kf cutoff," where kf is the Fermi wave vector. It is found that αm/ne and ωqm/ne1/3 are nearly constant. The αm ˜ ne can be used to identify the 3DDS phase as it differs from αm ˜ ne1/3 dependence in conventional bulk Cd3As2 semiconductor.
Acoustic phonon dynamics in thin-films of the topological insulator Bi{sub 2}Se{sub 3}
Glinka, Yuri D.; Babakiray, Sercan; Johnson, Trent A.; Holcomb, Mikel B.; Lederman, David
2015-04-28
Transient reflectivity traces measured for nanometer-sized films (6–40 nm) of the topological insulator Bi{sub 2}Se{sub 3} revealed GHz-range oscillations driven within the relaxation of hot carriers photoexcited with ultrashort (∼100 fs) laser pulses of 1.51 eV photon energy. These oscillations have been suggested to result from acoustic phonon dynamics, including coherent longitudinal acoustic phonons in the form of standing acoustic waves. An increase of oscillation frequency from ∼35 to ∼70 GHz with decreasing film thickness from 40 to 15 nm was attributed to the interplay between two different regimes employing traveling-acoustic-waves for films thicker than 40 nm and the film bulk acoustic wave resonator (FBAWR) modes for films thinner than 40 nm. The amplitude of oscillations decays rapidly for films below 15 nm thick when the indirect intersurface coupling in Bi{sub 2}Se{sub 3} films switches the FBAWR regime to that of the Lamb wave excitation. The frequency range of coherent longitudinal acoustic phonons is in good agreement with elastic properties of Bi{sub 2}Se{sub 3}.
Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites
Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W.; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin
2017-01-01
The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA+/MA+/Cs+, X=I−/Br−) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials. PMID:28106061
Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites.
Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin
2017-01-20
The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA(+)/MA(+)/Cs(+), X=I(-)/Br(-)) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials.
Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites
NASA Astrophysics Data System (ADS)
Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W.; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin
2017-01-01
The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA+/MA+/Cs+, X=I-/Br-) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials.
Zhao, J.; Boyko, O.; Bonello, B.
2014-12-15
This work deals with an analytical and numerical study of the focusing of the lowest order anti-symmetric Lamb wave in gradient index phononic crystals. Computing the ray trajectories of the elastic beam allowed us to analyze the lateral dimensions and shape of the focus, either in the inner or behind the phononic crystal-based acoustic lenses, for frequencies within a broad range in the first band. We analyzed and discussed the focusing behaviors inside the acoustic lenses where the focalization at sub-wavelength scale was achieved. The focalization behind the gradient index phononic crystal is shown to be efficient as well: we report on FMHM = 0.63λ at 11MHz.
NASA Astrophysics Data System (ADS)
Xie, Zhong-Xiang; Liu, Jing-Zhong; Yu, Xia; Wang, Hai-Bin; Deng, Yuan-Xiang; Li, Ke-Min; Zhang, Yong
2015-03-01
We investigate acoustic phonon transmission and thermal conductance in three dimensional (3D) quasi-periodically stubbed waveguides according to the Fibonacci sequence. Results show that the transmission coefficient exhibits the periodic oscillation upon varying the length of stub/waveguide at low frequency, and the period of such oscillation is tunably decreased with increasing the Fibonacci number N. Interestingly, there also exist some anti-resonant dips that gradually develop into wide stop-frequency gaps with increasing N. As the temperature goes up, a transition of the thermal conductance from the decrease to the increase occurs in these systems. When N is increased, the thermal conductance is approximately decreased with a linear trend. Moreover, the decreasing degree sensitively depends on the variation of temperature. A brief analysis of these results is given.
Investigation of phononic crystals for dispersive surface acoustic wave ozone sensors
NASA Astrophysics Data System (ADS)
Westafer, Ryan S.
The object of this research was to investigate dispersion in surface phononic crystals (PnCs) for application to a newly developed passive surface acoustic wave (SAW) ozone sensor. Frequency band gaps and slow sound already have been reported for PnC lattice structures. Such engineered structures are often advertised to reduce loss, increase sensitivity, and reduce device size. However, these advances have not yet been realized in the context of surface acoustic wave sensors. In early work, we computed SAW dispersion in patterned surface structures and we confirmed that our finite element computations of SAW dispersion in thin films and in one dimensional surface PnC structures agree with experimental results obtained by laser probe techniques. We analyzed the computations to guide device design in terms of sensitivity and joint spectral operating point. Next we conducted simulations and experiments to determine sensitivity and limit of detection for more conventional dispersive SAW devices and PnC sensors. Finally, we conducted extensive ozone detection trials on passive reflection mode SAW devices, using distinct components of the time dispersed response to compensate for the effect of temperature. The experimental work revealed that the devices may be used for dosimetry applications over periods of several days.
Development of an acoustic filter for parametric loudspeaker using phononic crystals.
Ji, Peifeng; Hu, Wenlin; Yang, Jun
2016-04-01
The spurious signal generated as a result of nonlinearity at the receiving system affects the measurement of the difference-frequency sound in the parametric loudspeaker, especially in the nearfield or near the beam axis. In this paper, an acoustic filter is designed using phononic crystals and its theoretical simulations are carried out by quasi-one- and two-dimensional models with Comsol Multiphysics. According to the simulated transmission loss (TL), an acoustic filter is prototyped consisting of 5×7 aluminum alloy cylinders and its performance is verified experimentally. There is good agreement with the simulation result for TL. After applying our proposed filter in the axial measurement of the parametric loudspeaker, a clear frequency dependence from parametric array effect is detected, which exhibits a good match with the well-known theory described by the Gaussian-beam expansion technique. During the directivity measurement for the parametric loudspeaker, the proposed filter has also proved to be effective and is only needed for small angles.
NASA Astrophysics Data System (ADS)
Pandya, Ankur; Jha, Prafulla K.
2017-04-01
Electron transport parameters such as electron effective mass, Fermi velocity of an electron and electron mobility are calculated for transition metal [manganese (Mn), cobalt (Co)]-doped armchair graphene nanoribbon (aGNR) via polar acoustical phonon [piezoelectric (PZ)] scattering and acoustical deformation potential (ADP) scattering under a high electric field and different doping concentrations. Moreover, the effect of dopant site on these electron transport parameters is also investigated. It is observed that the electron effective mass is reduced significantly in doped aGNR in comparison to pure GNR. It is observed that the net electron mobility contributed by both ADP and PZ mechanisms for Mn-doped aGNR as well as Co-doped aGNR varies in similar fashion as semiconductors wherein the net electron mobility (ADP + PZ) for Mn-doped aGNR is greater than that for the Co-doped graphene nanoribbon. Moreover, it is found that there is no impact of variation in dopant site on the electron transport parameters considered in this study.
NASA Astrophysics Data System (ADS)
Yang, Aichao; Li, Ping; Wen, Yumei; Yang, Chao; Wang, Decai; Zhang, Feng; Zhang, Jiajia
2015-05-01
A high-Q cross-plate phononic crystal resonator (Cr-PCR) coupled with an electromechanical Helmholtz resonator (EMHR) is proposed to improve acoustic wave localization and energy harvesting. Owing to the strongly directional wave-scattering effect of the cross-plate corners, strong confinement of acoustic waves emerges. Consequently, the proposed Cr-PCR structure exhibits ∼353.5 times higher Q value and ∼6.1 times greater maximum pressure amplification than the phononic crystal resonator (Cy-PCR) (consisting of cylindrical scatterers) of the same size. Furthermore, the harvester using the proposed Cr-PCR and the EMHR has ∼22 times greater maximum output-power volume density than the previous harvester using Cy-PCR and EMHR structures.
Carvalho, Bruno R; Wang, Yuanxi; Mignuzzi, Sandro; Roy, Debdulal; Terrones, Mauricio; Fantini, Cristiano; Crespi, Vincent H; Malard, Leandro M; Pimenta, Marcos A
2017-03-09
Double-resonance Raman scattering is a sensitive probe to study the electron-phonon scattering pathways in crystals. For semiconducting two-dimensional transition-metal dichalcogenides, the double-resonance Raman process involves different valleys and phonons in the Brillouin zone, and it has not yet been fully understood. Here we present a multiple energy excitation Raman study in conjunction with density functional theory calculations that unveil the double-resonance Raman scattering process in monolayer and bulk MoS2. Results show that the frequency of some Raman features shifts when changing the excitation energy, and first-principle simulations confirm that such bands arise from distinct acoustic phonons, connecting different valley states. The double-resonance Raman process is affected by the indirect-to-direct bandgap transition, and a comparison of results in monolayer and bulk allows the assignment of each Raman feature near the M or K points of the Brillouin zone. Our work highlights the underlying physics of intervalley scattering of electrons by acoustic phonons, which is essential for valley depolarization in MoS2.
Carvalho, Bruno R.; Wang, Yuanxi; Mignuzzi, Sandro; Roy, Debdulal; Terrones, Mauricio; Fantini, Cristiano; Crespi, Vincent H.; Malard, Leandro M.; Pimenta, Marcos A.
2017-01-01
Double-resonance Raman scattering is a sensitive probe to study the electron-phonon scattering pathways in crystals. For semiconducting two-dimensional transition-metal dichalcogenides, the double-resonance Raman process involves different valleys and phonons in the Brillouin zone, and it has not yet been fully understood. Here we present a multiple energy excitation Raman study in conjunction with density functional theory calculations that unveil the double-resonance Raman scattering process in monolayer and bulk MoS2. Results show that the frequency of some Raman features shifts when changing the excitation energy, and first-principle simulations confirm that such bands arise from distinct acoustic phonons, connecting different valley states. The double-resonance Raman process is affected by the indirect-to-direct bandgap transition, and a comparison of results in monolayer and bulk allows the assignment of each Raman feature near the M or K points of the Brillouin zone. Our work highlights the underlying physics of intervalley scattering of electrons by acoustic phonons, which is essential for valley depolarization in MoS2. PMID:28276472
NASA Astrophysics Data System (ADS)
Carvalho, Bruno R.; Wang, Yuanxi; Mignuzzi, Sandro; Roy, Debdulal; Terrones, Mauricio; Fantini, Cristiano; Crespi, Vincent H.; Malard, Leandro M.; Pimenta, Marcos A.
2017-03-01
Double-resonance Raman scattering is a sensitive probe to study the electron-phonon scattering pathways in crystals. For semiconducting two-dimensional transition-metal dichalcogenides, the double-resonance Raman process involves different valleys and phonons in the Brillouin zone, and it has not yet been fully understood. Here we present a multiple energy excitation Raman study in conjunction with density functional theory calculations that unveil the double-resonance Raman scattering process in monolayer and bulk MoS2. Results show that the frequency of some Raman features shifts when changing the excitation energy, and first-principle simulations confirm that such bands arise from distinct acoustic phonons, connecting different valley states. The double-resonance Raman process is affected by the indirect-to-direct bandgap transition, and a comparison of results in monolayer and bulk allows the assignment of each Raman feature near the M or K points of the Brillouin zone. Our work highlights the underlying physics of intervalley scattering of electrons by acoustic phonons, which is essential for valley depolarization in MoS2.
NASA Astrophysics Data System (ADS)
Rury, Aaron S.; Sorenson, Shayne; Dawlaty, Jahan M.
2016-03-01
Organic materials that produce coherent lattice phonon excitations in response to external stimuli may provide next generation solutions in a wide range of applications. However, for these materials to lead to functional devices in technology, a full understanding of the possible driving forces of coherent lattice phonon generation must be attained. To facilitate the achievement of this goal, we have undertaken an optical spectroscopic study of an organic charge-transfer material formed from the ubiquitous reduction-oxidation pair hydroquinone and p-benzoquinone. Upon pumping this material, known as quinhydrone, on its intermolecular charge transfer resonance as well as an intramolecular resonance of p-benzoquinone, we find sub-cm-1 oscillations whose dispersion with probe energy resembles that of a coherent acoustic phonon that we argue is coherently excited following changes in the electron density of quinhydrone. Using the dynamical information from these ultrafast pump-probe measurements, we find that the fastest process we can resolve does not change whether we pump quinhydrone at either energy. Electron-phonon coupling from both ultrafast coherent vibrational and steady-state resonance Raman spectroscopies allows us to determine that intramolecular electronic excitation of p-benzoquinone also drives the electron transfer process in quinhydrone. These results demonstrate the wide range of electronic excitations of the parent of molecules found in many functional organic materials that can drive coherent lattice phonon excitations useful for applications in electronics, photonics, and information technology.
Acoustic phonon modes in asymmetric AlxGa1-xN/GaN/AlyGa1-yN quantum wells
NASA Astrophysics Data System (ADS)
Zan, Y. H.; Ban, S. L.; Chai, Y. J.; Qu, Y.
2017-02-01
Using an elastic continuum model, the dispersion relations and phonon modes of propagating, confined, half space and interface acoustic phonons in asymmetric AlxGa1-xN/GaN/Al1-yGayN quantum wells (QWs) have been solved theoretically with the varieties of Al components x and y. Contrary to the previous conclusions, some regulations for the existence of the above different acoustic phonons are revealed as well as the transition conditions among these modes are also discussed. With increase of wave vectors, the dispersion relations split into several groups. Because the classification of these groups is related to the eigen frequencies of bulk materials forming QWs, phonon modes in these groups will be confined or propagating in different layers of QWs. Furthermore, the gradients of the dispersion relations' asymptotes are the velocities of longitudinal and the transverse acoustic phonons propagating in bulk materials in turns. The properties of the dispersion relations and their phonon modes are also analyzed in depth based on the cut-off conditions. By the changing of Al components x and y, the bottom of these groups will be modified to adjust eigen frequencies of AlxGa1-xN or Al1-yGayN layers. But the propagation properties of acoustic phonon modes will remain unchanged in each section.
Modelling of acoustic waves propagating in nesting Fibonacci super-lattice phononic crystal
NASA Astrophysics Data System (ADS)
Zhao, Min; Qi, Hai-Feng; Xu, Jia-Hui; Xie, Ya-Zhuo; Zhang, Xing-Gan; Gao, Jian
2014-07-01
Herein, we report construction of one kind of nesting-Fibonacci-super-lattice phononic crystal, in which the super-lattice cell is a well-defined Fibonacci generation sequence. We present a comparative study on band-gap structures of acoustic waves propagating in one-dimensional, nesting Fibonacci-periodic structure and simple-periodic structure. We find that there are more band gaps in nesting Fibonacci super-lattice models, and that they present behavior different from the split-up of band gaps with different generation numbers. With the increase of generation number, more band gaps split and occur. Additionally, when generation number becomes larger, Bragg scattering becomes more significant: the characteristic curves become flatter and band gaps become wider. Furthermore, we study the effect of various parameters such as density, thickness and defects on band-gap structures. Our work is significant both for understanding the intrinsic physical properties of nesting Fibonacci sequences and for providing flexible choices to meet real engineering requirements.
Coherent acoustic phonons in YBa2Cu3O7/La1/3Ca2/3MnO3 superlattices
NASA Astrophysics Data System (ADS)
Li, Wei; He, Bin; Zhang, Chunfeng; Liu, Shenghua; Liu, Xiaoran; Middey, S.; Chakhalian, J.; Wang, Xiaoyong; Xiao, Min
2016-03-01
We investigate photo-induced coherent acoustic phonons in complex oxide superlattices consisting of high-Tc superconductor YBa2Cu3O7-x and ferromagnetic manganite La1/3Ca2/3MnO3 epitaxial layers with broadband pump-probe spectroscopy. Two oscillatory components have been observed in time-resolved differential reflectivity spectra. Based on the analysis, the slow oscillation mode with a frequency sensitive to the probe wavelength is ascribed to the stimulated Brillouin scattering due to the photon reflection by propagating train of coherent phonons. The fast oscillation mode with a probe-wavelength-insensitive frequency is attributed to the Bragg oscillations caused by specular phonon reflections at oxide interfaces or the electron-coupling induced modulation due to free carrier absorption in the metallic superlattices. Our findings suggest that oxide superlattice is an ideal system to tailor the coherent behaviors of acoustic phonons and to manipulate the thermal and acoustic properties.
NASA Astrophysics Data System (ADS)
Shinokita, Keisuke; Reimann, Klaus; Woerner, Michael; Elsaesser, Thomas; Hey, Rudolf; Flytzanis, Christos
2016-02-01
Sound amplification in an electrically biased superlattice (SL) is studied in optical experiments with 100 fs time resolution. Coherent SL phonons with frequencies of 40, 375, and 410 GHz give rise to oscillatory reflectivity changes. With currents from 0.5 to 1.3 A, the Fourier amplitude of the 410 GHz phonon increases by more than a factor of 2 over a 200 ps period. This amplification is due to stimulated Čerenkov phonon emission by electrons undergoing intraminiband transport. The gain coefficient of 8 ×103 cm-1 is reproduced by theoretical calculations and holds potential for novel sub-THz phonon emitters.
Acoustic-phonon-assisted quantum control of qubit states near the Si/SiO2 interface
NASA Astrophysics Data System (ADS)
Gou, Bing-Ping; Zhao, Peiji; Kong, Xiao-Jun
2013-10-01
The waiting time between load/initialization and readout of electron spin qubit is related to electron tunneling between the donor and Si/SiO2 interface. Impacts of energy valley interference in silicon, lattice temperature, and screening of metallic gate on the waiting time associated with acoustic-phonon-assisted electron tunneling have been investigated. The results show that interface valley-orbit coupling causes its oscillation with donor depth and the influence of gate screening is significant when the SiO2 thickness is smaller than 10 nm. Moreover, the influences of these factors are strongest at critical electric field.
Shinokita, Keisuke; Reimann, Klaus; Woerner, Michael; Elsaesser, Thomas; Hey, Rudolf; Flytzanis, Christos
2016-02-19
Sound amplification in an electrically biased superlattice (SL) is studied in optical experiments with 100 fs time resolution. Coherent SL phonons with frequencies of 40, 375, and 410 GHz give rise to oscillatory reflectivity changes. With currents from 0.5 to 1.3 A, the Fourier amplitude of the 410 GHz phonon increases by more than a factor of 2 over a 200 ps period. This amplification is due to stimulated Čerenkov phonon emission by electrons undergoing intraminiband transport. The gain coefficient of 8×10^{3} cm^{-1} is reproduced by theoretical calculations and holds potential for novel sub-THz phonon emitters.
Ultra-wide acoustic band gaps in pillar-based phononic crystal strips
NASA Astrophysics Data System (ADS)
Coffy, Etienne; Lavergne, Thomas; Addouche, Mahmoud; Euphrasie, Sébastien; Vairac, Pascal; Khelif, Abdelkrim
2015-12-01
An original approach for designing a one dimensional phononic crystal strip with an ultra-wide band gap is presented. The strip consists of periodic pillars erected on a tailored beam, enabling the generation of a band gap that is due to both Bragg scattering and local resonances. The optimized combination of both effects results in the lowering and the widening of the main band gap, ultimately leading to a gap-to-midgap ratio of 138%. The design method used to improve the band gap width is based on the flattening of phononic bands and relies on the study of the modal energy distribution within the unit cell. The computed transmission through a finite number of periods corroborates the dispersion diagram. The strong attenuation, in excess of 150 dB for only five periods, highlights the interest of such ultra-wide band gap phononic crystal strips.
Ultra-wide acoustic band gaps in pillar-based phononic crystal strips
Coffy, Etienne Lavergne, Thomas; Addouche, Mahmoud; Euphrasie, Sébastien; Vairac, Pascal; Khelif, Abdelkrim
2015-12-07
An original approach for designing a one dimensional phononic crystal strip with an ultra-wide band gap is presented. The strip consists of periodic pillars erected on a tailored beam, enabling the generation of a band gap that is due to both Bragg scattering and local resonances. The optimized combination of both effects results in the lowering and the widening of the main band gap, ultimately leading to a gap-to-midgap ratio of 138%. The design method used to improve the band gap width is based on the flattening of phononic bands and relies on the study of the modal energy distribution within the unit cell. The computed transmission through a finite number of periods corroborates the dispersion diagram. The strong attenuation, in excess of 150 dB for only five periods, highlights the interest of such ultra-wide band gap phononic crystal strips.
Observing backfolded and unfolded acoustic phonons by broadband optical light scattering.
Maerten, L; Bojahr, A; Bargheer, M
2015-02-01
We use broadband time domain Brillouin scattering to observe coherently generated phonon modes in bulk and nanolayered samples. We transform the measured transients into a frequency-wavevector diagram and compare the resulting dispersion relations to calculations. The detected oscillation amplitude depends on the occupation of phonon modes induced by the pump pulse. For nanolayered samples with an appropriately large period, the whole wavevector range of the Brillouin zone becomes observable by broadband optical light scattering. The backfolded modes vanish, when the excitation has passed the nanolayers and propagates through the substrate underneath.
Acoustic phonon-limited diffusion thermopower in monolayer MoS{sub 2}
Patil, S. B.; Sankeshwar, N. S. Kubakaddi, S. S.
2015-06-24
Diffusion thermopower S{sub d} is investigated, theoretically, as a function of temperature, T and electron concentration, n{sub s} in a n-type monolayer molebdenum disulfide (MoS{sub 2}). Electron scattering due to unscreened deformation potential (DP) coupling of TA phonons, screened DP coupling of LA phonons, and screened piezoelectric (PE) coupling of LA and TA phonons is considered. Total S{sub d} is dominated by electron scattering by TA phonons via unscreened DP coupling. S{sub d} is found to increase (decrease) with increasing T (n{sub s}). At low T and for high n{sub s}, S{sub d} ∼ T and n{sub s}{sup −1} as found from the Mott formula. At a given T and for given ns, S{sub d} in MoS{sub 2} is much larger than that in GaAs, due to the larger electron effective mass in the former.
NASA Technical Reports Server (NTRS)
Strekalov, Dmitry V.; Yu, Nan
2010-01-01
Optical sidebands have been generated with relative frequency tens to hundreds of GHz by using optical sidebands that are generated in a cascade process in high-quality optical resonators with Kerr nonlinearity, such as whispering gallery mode (WGM) resonators. For this purpose, the WGM resonator needs to be optically pumped at two frequencies matching its resonances. These two optical components can be one or several free spectral ranges (FSRs), equal to approximately 12 GHz, in this example, apart from each other, and can be easily derived from a monochromatic pump with an ordinary EOM (electro-optic modulation) operating at half the FSR frequency. With sufficient nonlinearity, an optical cascade process will convert the two pump frequencies into a comb-like structure extending many FSRs around the carrier frequency. This has a demonstratively efficient frequency conversion of this type with only a few milliwatt optical pump power. The concept of using Kerr nonlinearity in a resonator for non-degenerate wave mixing has been discussed before, but it was a common belief that this was a weak process requiring very high peak powers to be observable. It was not thought possible for this approach to compete with electro-optical modulators in CW applications, especially those at lower optical powers. By using the high-Q WGM resonators, the effective Kerr nonlinearity can be made so high that, using even weak seeding bands available from a conventional EOM, one can effectively multiply the optical sidebands, extending them into an otherwise inaccessible frequency range.
Lin, Kung-Hsuan; Wang, Kuan-Jen; Chang, Chung-Chieh; Wen, Yu-Chieh; Lv, Bing; Chu, Ching-Wu; Wu, Maw-Kuen
2016-01-01
We have utilized ultrafast optical spectroscopy to study carrier dynamics in slightly underdoped (BaK)Fe2As2 crystals without magnetic transition. The photoelastic signals due to coherent acoustic phonons have been quantitatively investigated. According to our temperature-dependent results, we found that the relaxation component of superconducting quasiparticles persisted from the superconducting state up to at least 70 K in the normal state. Our findings suggest that the pseudogaplike feature in the normal state is possibly the precursor of superconductivity. We also highlight that the pseudogap feature of K-doped BaFe2As2 is different from that of other iron-based superconductors, including Co-doped or P-doped BaFe2As2. PMID:27180873
Pollock, Kevin L; Doan, Hoang Q; Rustagi, Avinash; Stanton, Christopher J; Cuk, Tanja
2017-03-02
A prominent architecture for solar energy conversion layers diverse materials, such as traditional semiconductors (Si, III-V) and transition metal oxides (TMOs), into a monolithic device. The efficiency with which photoexcited carriers cross each layer is critical to device performance and dependent on the electronic properties of a heterojunction. Here, by time-resolved changes in the reflectivity after excitation of an n-GaAs/p-GaAs/TMO (Co3O4, IrO2) device, we detect a photoexcited carrier distribution specific to the p-GaAs/TMO interface through its coupling to phonons in both materials. The photoexcited carriers generate two coherent longitudinal acoustic phonons (CLAPs) traveling in opposite directions, one into the TMO and the other into the p-GaAs. This is the first time a CLAP is reported to originate at a semiconductor/TMO heterojunction. Therefore, these experiments seed future modeling of the built-in electric fields, the internal Fermi level, and the photoexcited carrier density of semiconductor/TMO interfaces within multilayered heterostructures.
Tunable broadband unidirectional acoustic transmission based on a waveguide with phononic crystal
NASA Astrophysics Data System (ADS)
Song, Ailing; Chen, Tianning; Wang, Xiaopeng; Wan, Lele
2016-08-01
In this paper, a tunable broadband unidirectional acoustic transmission (UAT) device composed of a bended tube and a superlattice with square columns is proposed and numerically investigated by using finite element method. The UAT is realized in the proposed UAT device within two wide frequency ranges. And the effectiveness of the UAT device is demonstrated by analyzing the sound pressure distributions when the acoustic waves are incident from different directions. The unidirectional band gaps can be effectively tuned by mechanically rotating the square columns, which is a highlight of this paper. Besides, a bidirectional acoustic isolation (BAI) device is obtained by placing two superlattices in the bended tube, in which the acoustic waves cannot propagate along any directions. The physical mechanisms of the proposed UAT device and BAI device are simply discussed. The proposed models show potential applications in some areas, such as unidirectional sonic barrier or noise insulation.
Phononic crystal surface mode coupling and its use in acoustic Doppler velocimetry.
Cicek, Ahmet; Salman, Aysevil; Kaya, Olgun Adem; Ulug, Bulent
2016-02-01
It is numerically shown that surface modes of two-dimensional phononic crystals, which are Bloch modes bound to the interface between the phononic crystal and the surrounding host, can couple back and forth between the surfaces in a length scale determined by the separation of two surfaces and frequency. Supercell band structure computations through the finite-element method reveal that the surface band of an isolated surface splits into two bands which support either symmetric or antisymmetric hybrid modes. When the surface separation is 3.5 times the lattice constant, a coupling length varying between 30 and 48 periods can be obtained which first increases linearly with frequency and, then, decreases rapidly. In the linear regime, variation of coupling length can be used as a means of measuring speeds of objects on the order of 0.1m/s by incorporating the Doppler shift. Speed sensitivity can be improved by increasing surface separation at the cost of larger device sizes.
NASA Astrophysics Data System (ADS)
Peelaers, H.; Partoens, B.; Peeters, F. M.
2009-09-01
The phonon spectra of thin freestanding, hydrogen passivated, Ge nanowires are calculated by ab initio techniques. The effect of confinement on the phonon modes as caused by the small diameters of the wires is investigated. Confinement causes a hardening of the optical modes and a softening of the longitudinal acoustic modes. The stability of the nanowires, undoped or doped with B or P atoms, is investigated using the obtained phonon spectra. All considered wires were stable, except for highly doped, very thin nanowires.
Lee, Sooheyong; Williams, G. Jackson; Campana, Maria I.; Walko, Donald A.; Landahl, Eric C.
2016-01-01
Using a strain-rosette, we demonstrate the existence of transverse strain using time-resolved x-ray diffraction from multiple Bragg reflections in laser-excited bulk gallium arsenide. We find that anisotropic strain is responsible for a considerable fraction of the total lattice motion at early times before thermal equilibrium is achieved. Our measurements are described by a new model where the Poisson ratio drives transverse motion, resulting in the creation of shear waves without the need for an indirect process such as mode conversion at an interface. Using the same excitation geometry with the narrow-gap semiconductor indium antimonide, we detected coherent transverse acoustic oscillations at frequencies of several GHz. PMID:26751616
Lee, Sooheyong; Williams, G. Jackson; Campana, Maria I.; Walko, Donald A.; Landahl, Eric C.
2016-01-11
Using a strain-rosette, we demonstrate the existence of transverse strain using time-resolved x-ray diffraction from multiple Bragg reflections in laser-excited bulk gallium arsenide. We find that anisotropic strain is responsible for a considerable fraction of the total lattice motion at early times before thermal equilibrium is achieved. Our measurements are described by a new model where the Poisson ratio drives transverse motion, resulting in the creation of shear waves without the need for an indirect process such as mode conversion at an interface. Finally, using the same excitation geometry with the narrow-gap semiconductor indium antimonide, we detected coherent transverse acoustic oscillations at frequencies of several GHz.
NASA Astrophysics Data System (ADS)
Andronikova, D. A.; Bronwald, I. A.; Burkovsky, R. G.; Leontiev, I. N.; Leontiev, N. G.; Bosak, A. A.; Filimonov, A. V.; Vakhrushev, S. B.
2016-11-01
Inelastic X-ray scattering measurements have been done to study the lattice dynamics in lead zirconate titanate solid solution with 0.7% of PbTiO3. The temperature evolution of central peak and low-energy transverse phonon branches has been traced. Temperature dependent in-plane transverse polarized acoustic phonon branch in <1 1 0> direction has been revealed. The central peaks of two types have been found. The central peak at small wave vectors can be attributed to the relaxational-type soft ferroelectric mode, while the latter at Q = (1.5 -0.5 0) could be linked to the formation of M-superstructure in the intermediate ferroelectric phase.
Biswas, Tutul; Ghosh, Tarun Kanti
2013-01-23
We study the interaction between electron and acoustic phonons in a Rashba spin-orbit coupled two-dimensional electron gas using Boltzmann transport theory. Both the deformation potential and piezoelectric scattering mechanisms are considered in the Bloch-Grüneisen (BG) regime as well as in the equipartition (EP) regime. The effect of the Rashba spin-orbit interaction on the temperature dependence of the resistivity in the BG and EP regimes is discussed. We find that the effective exponent of the temperature dependence of the resistivity in the BG regime decreases due to spin-orbit coupling.
Phonon dispersion in hypersonic two-dimensional phononic crystal membranes
NASA Astrophysics Data System (ADS)
Graczykowski, B.; Sledzinska, M.; Alzina, F.; Gomis-Bresco, J.; Reparaz, J. S.; Wagner, M. R.; Sotomayor Torres, C. M.
2015-02-01
We investigate experimentally and theoretically the acoustic phonon propagation in two-dimensional phononic crystal membranes. Solid-air and solid-solid phononic crystals were made of square lattices of holes and Au pillars in and on 250 nm thick single crystalline Si membrane, respectively. The hypersonic phonon dispersion was investigated using Brillouin light scattering. Volume reduction (holes) or mass loading (pillars) accompanied with second-order periodicity and local resonances are shown to significantly modify the propagation of thermally activated GHz phonons. We use numerical modeling based on the finite element method to analyze the experimental results and determine polarization, symmetry, or three-dimensional localization of observed modes.
Nonlinear phononics using atomically thin membranes
NASA Astrophysics Data System (ADS)
Midtvedt, Daniel; Isacsson, Andreas; Croy, Alexander
2014-09-01
Phononic crystals and acoustic metamaterials are used to tailor phonon and sound propagation properties by utilizing artificial, periodic structures. Analogous to photonic crystals, phononic band gaps can be created, which influence wave propagation and, more generally, allow engineering of the acoustic properties of a system. Beyond that, nonlinear phenomena in periodic structures have been extensively studied in photonic crystals and atomic Bose-Einstein condensates in optical lattices. However, creating nonlinear phononic crystals or nonlinear acoustic metamaterials remains challenging and only few examples have been demonstrated. Here, we show that atomically thin and periodically pinned membranes support coupled localized modes with nonlinear dynamics. The proposed system provides a platform for investigating nonlinear phononics.
NASA Astrophysics Data System (ADS)
Fobes, David; Zaliznyak, Igor; Xu, Zhijun; Gu, Genda; Tranquada, John M.; He, Xu-Gang; Ku, Wei; Garlea, Ovidiu
2014-03-01
We have studied the evolution with temperature of the low-energy inelastic spectra of Fe1+yTe (y < 0 . 12), a parent compound of the iron-chalcogenide superconductor family, revealing an acoustic mode at an unexpected position. Recently, we found evidence for the formation of a bond-order wave leading to ferro-orbital order in the monoclinic phase, in part due to the observation of an elastic structural peak at (100) in the low-temperature monoclinic phase [D. Fobes, et al., arXiv:1307.7162]. In the inelastic spectra we observe a sharp acoustic-phonon-like mode dispersing out of the (100) position in the monoclinic phase. Surprisingly, the mode survives in the tetragonal phase, despite the absence of a Bragg peak at (100); such a peak is forbidden by symmetry. LDA calculations suggest this mode could involve significant magnetic scattering. By assuming in-phase virtual displacement of the Fe atoms from their equilibrium position in a frozen phonon calculation, we have found a small but significant imbalance in the magnetic moments between the two Fe atoms within the unit cell, suggesting magnetic contribution to the mode. Work at BNL supported by Office of Basic Energy Sciences, US DOE, under Contract No. DE-AC02-98CH10886. Research conducted at ORNL Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US DOE.
NASA Astrophysics Data System (ADS)
Toulouse, J.; Iolin, E.; Hennion, B.; Petitgrand, D.; Erwin, R.
2016-12-01
The damping (Γ a ) of the transverse acoustic (TA) phonon in single crystals of the relaxor KT a1 -xN bxO3 with x =0.15 -0.17 was studied by means of high resolution inelastic cold neutron scattering near the (200) Brillouin Zone (BZ) point where diffuse scattering is absent, although it is present near (110). In a wide range of temperatures centered on the phase transition, T =195 K ÷108 K , the TA phonon width (damping) exhibits a step increase around momentum q =0.07 , goes through a shallow maximum at q =0.09 -0.12 , and remains high above and up to the highest momentum studied of q =0.16 . These experimental results are explained in terms of a resonant interaction between the TA phonon and the collective or correlated reorientation through tunneling of the off-center N b+5 ions. The observed TA damping is successfully reproduced in a simple model that includes an interaction between the TA phonon and a dispersionless localized mode (LM) with frequency ωL and damping ΓL(ΓL<ωL) , itself coupled to the transverse optic (TO) mode. Maximum damping of the TA phonon occurs when its frequency is ωa≈ωL . The values of ωL and ΓL are moderately dependent on temperature, but the oscillator strength, M2, of the resonant damping exhibits a strong maximum in the range T ˜120 K ÷150 K in which neutron diffuse scattering near the (110) BZ point is also maximum and the dielectric susceptibility exhibits the relaxor behavior. The maximum value of M appears to be due to the increasing number of polar nanodomains. In support of the proposed model, the observed value of ωL≈0.7 THz is found to be similar to the estimate previously obtained by Girshberg and Yacoby [J. Phys.: Condens. Matter 24, 015901 (2012)], 10.1088/0953-8984/24/1/015901. Alternatively, the TA phonon damping can be successfully fitted in the framework of an empirical Havriliak-Negami (HN) relaxation model that includes a strong resonancelike transient contribution.
Nakayama, Masaaki Ohno, Tatsuya; Furukawa, Yoshiaki
2015-04-07
We have systematically investigated the photoluminescence (PL) dynamics of free excitons in GaAs/Al{sub 0.3}Ga{sub 0.7}As single quantum wells, focusing on the energy relaxation process due to exciton–acoustic-phonon scattering under non-resonant and weak excitation conditions as a function of GaAs-layer thickness from 3.6 to 12.0 nm and temperature from 30 to 50 K. The free exciton characteristics were confirmed by observation that the PL decay time has a linear dependence with temperature. We found that the free exciton PL rise rate, which is the reciprocal of the rise time, is inversely linear with the GaAs-layer thickness and linear with temperature. This is consistent with a reported theoretical study of the exciton–acoustic-phonon scattering rate in the energy relaxation process in quantum wells. Consequently, it is conclusively verified that the PL rise rate is dominated by the exciton–acoustic-phonon scattering rate. In addition, from quantitative analysis of the GaAs-layer thickness and temperature dependences, we suggest that the PL rise rate reflects the number of exciton–acoustic-phonon scattering events.
Bhargavi, K. S.; Patil, Sukanya; Kubakaddi, S. S.
2015-07-28
The theory of free-carrier absorption (FCA) is given for monolayers of transition-metal dichalcogenides, particularly for molybdenum disulphide (MoS{sub 2}), when carriers are scattered by phonons. Explicit expressions for the absorption coefficient α are obtained and discussed for acoustic phonon scattering via screened deformation potential and piezoelectric coupling taking polarization of the radiation in the plane of the layer. It is found that α monotonously decreases with the increasing photon frequency Ω, increases with the increasing temperature T, and linearly depends on two-dimensional electron concentration n{sub s}. Effect of screening, which is ignored in all the earlier FCA studies, is found to reduce α significantly, attributing to the larger effective mass of the electrons. Results are also obtained in the classical and quantum limit giving the power laws α ∼ Ω{sup −2} and T. Comparison of the results is made with those in bulk semiconductors and semiconductor quantum wells.
Roy, C; Hughes, S
2011-06-17
We study the resonance fluorescence spectra of a driven quantum dot placed inside a high-Q semiconductor cavity and interacting with an acoustic phonon bath. The dynamics is calculated using a time-convolutionless master equation in the polaron frame. We predict pronounced spectral broadening of the Mollow sidebands through off-resonant cavity emission which, for small cavity-coupling rates, increases quadratically with the Rabi frequency in direct agreement with recent experiments using semiconductor micropillars [S. M. Ulrich et al., preceding Letter, Phys. Rev. Lett. 106, 247402 (2011)]. We also demonstrate that, surprisingly, phonon coupling actually helps resolve signatures of the elusive second rungs of the Jaynes-Cummings ladder states via off-resonant cavity feeding. Both multiphonon and multiphoton effects are shown to play a qualitatively important role on the fluorescence spectra.
Minimize reference sideband generation in microwave PLLs
NASA Astrophysics Data System (ADS)
Goldman, Stan
1991-02-01
The processes responsible for producing reference sidebands are outlined, and the sources of coupling to the microwave voltage-controlled oscillator (VCO) tune line including power-supply-generated signals, TTL-controlled interface signals, intermediate programmable-divider signals, and radiated TTL signals are discussed. It is noted that filtering alone is inadequate for reference-sideband suppression, while minimizing the tuning slope and maximizing the reference frequency will result in a reduced reference-sideband level. Minimizing offset currents by using a differential amplifier connection may reduce the reference-sideband level aggravated by an opamp. The selection of a TTL, ECL, or GaAs phase/frequency detector can determine the level of reference sidebands, as well as PCB isolation techniques.
Phononic crystal diffraction gratings
NASA Astrophysics Data System (ADS)
Moiseyenko, Rayisa P.; Herbison, Sarah; Declercq, Nico F.; Laude, Vincent
2012-02-01
When a phononic crystal is interrogated by an external source of acoustic waves, there is necessarily a phenomenon of diffraction occurring on the external enclosing surfaces. Indeed, these external surfaces are periodic and the resulting acoustic diffraction grating has a periodicity that depends on the orientation of the phononic crystal. This work presents a combined experimental and theoretical study on the diffraction of bulk ultrasonic waves on the external surfaces of a 2D phononic crystal that consists of a triangular lattice of steel rods in a water matrix. The results of transmission experiments are compared with theoretical band structures obtained with the finite-element method. Angular spectrograms (showing frequency as a function of angle) determined from diffraction experiments are then compared with finite-element simulations of diffraction occurring on the surfaces of the crystal. The experimental results show that the diffraction that occurs on its external surfaces is highly frequency-dependent and has a definite relation with the Bloch modes of the phononic crystal. In particular, a strong influence of the presence of bandgaps and deaf bands on the diffraction efficiency is found. This observation opens perspectives for the design of efficient phononic crystal diffraction gratings.
Splash, pop, sizzle: Information processing with phononic computing
Sklan, Sophia R.
2015-05-15
Phonons, the quanta of mechanical vibration, are important to the transport of heat and sound in solid materials. Recent advances in the fundamental control of phonons (phononics) have brought into prominence the potential role of phonons in information processing. In this review, the many directions of realizing phononic computing and information processing are examined. Given the relative similarity of vibrational transport at different length scales, the related fields of acoustic, phononic, and thermal information processing are all included, as are quantum and classical computer implementations. Connections are made between the fundamental questions in phonon transport and phononic control and the device level approach to diodes, transistors, memory, and logic. .
Enhanced electron-phonon coupling for a semiconductor charge qubit in a surface phonon cavity
Chen, J. C. H.; Sato, Y.; Kosaka, R.; Hashisaka, M.; Muraki, K.; Fujisawa, T.
2015-01-01
Electron-phonon coupling is a major decoherence mechanism, which often causes scattering and energy dissipation in semiconductor electronic systems. However, this electron-phonon coupling may be used in a positive way for reaching the strong or ultra-strong coupling regime in an acoustic version of the cavity quantum electrodynamic system. Here we propose and demonstrate a phonon cavity for surface acoustic waves, which is made of periodic metal fingers that constitute Bragg reflectors on a GaAs/AlGaAs heterostructure. Phonon band gap and cavity phonon modes are identified by frequency, time and spatially resolved measurements of the piezoelectric potential. Tunneling spectroscopy on a double quantum dot indicates the enhancement of phonon assisted transitions in a charge qubit. This encourages studying of acoustic cavity quantum electrodynamics with surface phonons. PMID:26469629
NASA Astrophysics Data System (ADS)
Salman, Aysevil; Adem Kaya, Olgun; Cicek, Ahmet; Ulug, Bulent
2015-06-01
Mach-Zehnder interferometer formed by liquid-filled linear defect waveguides in a two-dimensional phononic crystal is numerically realized for sensing low concentrations of an analyte. The waveguides in the square phononic crystal of void cylinders in steel, as well as their T branches and sharp bends are utilized to construct interferometer arms. Sensing low concentrations of ethanol on the order of 0.1% in a binary mixture with water is achieved by replacing the contents of a number of waveguide core cells on one arm of the interferometer with the analyte. Computations are carried out through the finite-element method in an approach that takes the solid-liquid interaction at the waveguide core cells into account. Band analyses reveal linear variation of the central frequency of the transmission band within a band gap for ethanol concentrations up to 3.0%. Phase difference due to the imbalance of the sample and reference arms of the interferometer also varies linearly with ethanol concentration, leading in turn to a cosine variation of the Fourier component of the temporal interferometer response at the central input-pulse frequency. The induced phase difference in the investigated configuration becomes a -0.78π and -0.65π per percent increase of ethanol concentration as calculated from the band-structure and transient data, respectively. This is confirmed by transient finite-element simulations where totally destructive interference occurs for a concentration of approximately 1.5%. The proposed scheme, which can easily be adopted to other binary mixtures, offers a compact implementation requiring small amounts of analyte.
NASA Astrophysics Data System (ADS)
Børkje, Kjetil
2016-10-01
We consider a system where an optical cavity mode is parametrically coupled to a mechanical oscillator. A laser beam driving the cavity at its resonance frequency will acquire red- and blue-shifted sidebands due to noise in the position of the mechanical oscillator. In a classical theory without noise in the electromagnetic field, the powers of these sidebands are of equal magnitude. In a quantum theory, however, an asymmetry between the sidebands can be resolved when the oscillator's average number of vibrational excitations (phonons) becomes small, i.e., comparable to 1. We discuss the interpretation of this sideband asymmetry in a heterodyne photodetection measurement scheme and show that it depends on the choice of detector model. In the optical regime, standard photodetection theory leads to a photocurrent noise spectrum given by normal- and time-ordered expectation values. The sideband asymmetry is in that case a direct reflection of the quantum asymmetry of the position noise spectrum of the mechanical oscillator. Conversely, for a detector that measures symmetric, nonordered expectation values, we show that the sideband asymmetry can be traced back to quantum optomechanical interference terms. This ambiguity in interpretation applies not only to mechanical oscillators, but to any degree of freedom that couples linearly to noise in the electromagnetic field. Finally, we also compare the quantum theory to a fully classical model, where sideband asymmetry can arise from classical optomechanical interference terms. We show that, due to the oscillator's lack of zero-point motion in a classical theory, the sidebands in the photocurrent spectrum differ qualitatively from those of a quantum theory at sufficiently low temperatures. We discuss the observable consequences of this deviation between classical and quantum theories.
NASA Astrophysics Data System (ADS)
Zhang, Heng; Yu, SiYuan; Liu, FuKang; Wang, Zhen; Lu, MingHui; Hu, XiaoBo; Chen, YanFeng; Xu, XianGang
2017-04-01
The propagation of surface acoustic waves (SAWs) in two-dimensional phononic crystals (PnCs) with and without coupling-enhancement slabs was theoretically investigated using a three-dimensional finite element method. Different piezoelectric substrates, for example, lithium niobate (LiNbO3), gallium nitride (GaN), and aluminium nitride (AlN), were taken into account. Compared to the PnCs without coupling-enhancement slabs, the coupling between each pillar and its nearest neighbor was largely enhanced in the presence of slabs. The bandwidth of the first directional band gap increased markedly compared with its initial value for the PnCs without a slab (within square symmetry). In addition, with increasing thicknesses of the slabs bonded between neighboring pillars, the first directional band-gap and second directional band gap of the PnCs tend to merge. Therefore, the structure with coupling-enhancement slabs can be used as an excellent electrical band elimination filter for most electro-SAW devices, offering a new strategy to realize chip-scale applications in electroacoustic signal processing, optoacoustic modulation, and even SAW microfluidic devices.
Phonon-assisted gain in a semiconductor double quantum dot maser.
Gullans, M J; Liu, Y-Y; Stehlik, J; Petta, J R; Taylor, J M
2015-05-15
We develop a microscopic model for the recently demonstrated double-quantum-dot maser. In characterizing the gain of this device we find that, in addition to the direct stimulated emission of photons, there is a large contribution from the simultaneous emission of a photon and a phonon, i.e., the phonon sideband. We show that this phonon-assisted gain typically dominates the overall gain, which leads to masing. Recent experimental data are well fit with our model.
Sound and heat revolutions in phononics.
Maldovan, Martin
2013-11-14
The phonon is the physical particle representing mechanical vibration and is responsible for the transmission of everyday sound and heat. Understanding and controlling the phononic properties of materials provides opportunities to thermally insulate buildings, reduce environmental noise, transform waste heat into electricity and develop earthquake protection. Here I review recent progress and the development of new ideas and devices that make use of phononic properties to control both sound and heat. Advances in sonic and thermal diodes, optomechanical crystals, acoustic and thermal cloaking, hypersonic phononic crystals, thermoelectrics, and thermocrystals herald the next technological revolution in phononics.
NASA Astrophysics Data System (ADS)
Perrin, Bernard
2007-06-01
The conference PHONONS 2007 was held 15-20 July 2007 in the Conservatoire National des Arts et Métiers (CNAM) Paris, France. CNAM is a college of higher technology for training students in the application of science to industry, founded by Henri Grégoire in 1794. This was the 12th International Conference on Phonon Scattering in Condensed Matter. This international conference series, held every 3 years, started in France at Sainte-Maxime in 1972. It was then followed by meetings at Nottingham (1975), Providence (1979), Stuttgart (1983), Urbana-Champaign (1986), Heidelberg (1989), Ithaca (1992), Sapporo (1995), Lancaster (1998), Dartmouth (2001) and St Petersburg (2004). PHONONS 2007 was attended by 346 delegates from 37 different countries as follows: France 120, Japan 45, Germany 25, USA 25, Russia 21, Italy 13, Poland 9, UK 9, Canada 7, The Netherlands 7, Finland 6, Spain 6, Taiwan 6, Greece 4, India 4, Israel 4, Ukraine 4, Serbia 3, South Africa 3, Argentina 2, Belgium 2, China 2, Iran 2, Korea 2, Romania 2, Switzerland 2, and one each from Belarus, Bosnia-Herzegovina, Brazil, Bulgaria, Egypt, Estonia, Mexico, Moldova, Morocco, Saudi Arabia, Turkey. There were 5 plenary lectures, 14 invited talks and 84 oral contributions; 225 posters were presented during three poster sessions. The first plenary lecture was given by H J Maris who presented fascinating movies featuring the motion of a single electron in liquid helium. Robert Blick gave us a review on the new possibilities afforded by nanotechnology to design nano-electomechanical systems (NEMS) and the way to use them to study elementary and fundamental processes. The growing interest for phonon transport studies in nanostructured materials was demonstrated by Arun Majumdar. Andrey Akimov described how ultrafast acoustic solitons can monitor the optical properties of quantum wells. Finally, Maurice Chapellier told us how
Phonons in twisted bilayer graphene
NASA Astrophysics Data System (ADS)
Cocemasov, Alexandr I.; Nika, Denis L.; Balandin, Alexander A.
2013-07-01
We theoretically investigate phonon dispersion in AA-stacked, AB-stacked, and twisted bilayer graphene with various rotation angles. The calculations are performed using the Born-von Karman model for the intralayer atomic interactions and the Lennard-Jones potential for the interlayer interactions. It is found that the stacking order affects the out-of-plane acoustic phonon modes the most. The difference in the phonon densities of states in the twisted bilayer graphene and in AA- or AB-stacked bilayer graphene appears in the phonon frequency range 90-110 cm-1. Twisting bilayer graphene leads to the emergence of different phonon branches—termed hybrid folded phonons—which originate from the mixing of phonon modes from different high-symmetry directions in the Brillouin zone. The frequencies of the hybrid folded phonons depend strongly on the rotation angle and can be used for noncontact identification of the twist angles in graphene samples. The obtained results and the tabulated frequencies of phonons in twisted bilayer graphene are important for the interpretation of experimental Raman data and in determining the thermal conductivity of these material systems.
Xu, Yuehua; Dai, Jun; Zeng, Xiao Cheng
2016-01-21
The intrinsic acoustic-phonon-limited carrier mobility (μ) of Al2C monolayer sheet and nanoribbons are investigated using ab initio computation and deformation potential theory. It is found that the polarity of the room-temperature carrier mobility of the Al2C monolayer is direction-dependent, with μ of electron (e) and hole (h) being 2348 and 40.77 cm(2)/V/s, respectively, in the armchair direction and 59.95 (e) and 705.8 (h) in the zigzag direction. More interestingly, one-dimensional Al2C nanoribbons not only can retain the direction-dependent polarity but also may entail even higher mobility, in contrast to either the graphene nanoribbons which tend to exhibit lower μ compared to the two-dimensional graphene or the MoS2 nanoribbons which have reversed polarity compared to the MoS2 sheet. As an example, the Al-terminated zigzag nanoribbon with a width of 4.1 nm exhibits μ of 212.6 (e) and 2087 (h) cm(2)/V/s, while the C-terminated armchair nanoribbon with a width 2.6 nm exhibits μ of 1090 (e) and 673.9 (h) cm(2)/V/s; the C-terminated zigzag nanoribbon with a width 3.7 nm exhibits μ of 177.6 (e) and 1889 (h) cm(2)/V/s, and the Al-terminated armchair nanoribbon with a width 2.4 nm exhibits μ of 6695 (e) and 518.4 (h) cm(2)/V/s. The high carrier mobility, μ, coupled with polarity and direction dependence endows the Al2C sheet and nanoribbons with unique transport properties that can be exploited for special applications in nanoelectronics.
Microfabricated phononic crystal devices and applications
NASA Astrophysics Data System (ADS)
Olsson, R. H., III; El-Kady, I.
2009-01-01
Phononic crystals are the acoustic wave analogue of photonic crystals. Here a periodic array of scattering inclusions located in a homogeneous host material forbids certain ranges of acoustic frequencies from existence within the crystal, thus creating what are known as acoustic bandgaps. The majority of previously reported phononic crystal devices have been constructed by hand, assembling scattering inclusions in a viscoelastic medium, predominantly air, water or epoxy, resulting in large structures limited to frequencies below 1 MHz. Recently, phononic crystals and devices have been scaled to VHF (30-300 MHz) frequencies and beyond by utilizing microfabrication and micromachining technologies. This paper reviews recent developments in the area of micro-phononic crystals including design techniques, material considerations, microfabrication processes, characterization methods and reported device structures. Micro-phononic crystal devices realized in low-loss solid materials are emphasized along with their potential application in radio frequency communications and acoustic imaging for medical ultrasound and nondestructive testing. The reported advances in batch micro-phononic crystal fabrication and simplified testing promise not only the deployment of phononic crystals in a number of commercial applications but also greater experimentation on a wide variety of phononic crystal structures.
Slow light and broadband coherent phonon generation
NASA Astrophysics Data System (ADS)
Wang, Zheng; Rakich, Peter; Reinke, Charles; Camacho, Ryan; Davids, Paul
2012-03-01
Recent advance in controlling optical forces using nanostructures suggests that nanoscale optical waveguides are capable of generating coherent acoustic phonons efficiently through a combination of radiation pressure and electrostriction. We discuss the critical roles of group velocity in such processes. This photon-phonon coupling would allow an acoustic intermediary to perform on-chip optical delay with a capacity 105 greater than photonic delay lines of the same size.
Coherent phonon optics in a chip with an electrically controlled active device.
Poyser, Caroline L; Akimov, Andrey V; Campion, Richard P; Kent, Anthony J
2015-02-05
Phonon optics concerns operations with high-frequency acoustic waves in solid media in a similar way to how traditional optics operates with the light beams (i.e. photons). Phonon optics experiments with coherent terahertz and sub-terahertz phonons promise a revolution in various technical applications related to high-frequency acoustics, imaging, and heat transport. Previously, phonon optics used passive methods for manipulations with propagating phonon beams that did not enable their external control. Here we fabricate a phononic chip, which includes a generator of coherent monochromatic phonons with frequency 378 GHz, a sensitive coherent phonon detector, and an active layer: a doped semiconductor superlattice, with electrical contacts, inserted into the phonon propagation path. In the experiments, we demonstrate the modulation of the coherent phonon flux by an external electrical bias applied to the active layer. Phonon optics using external control broadens the spectrum of prospective applications of phononics on the nanometer scale.
Coherent phonon optics in a chip with an electrically controlled active device
Poyser, Caroline L.; Akimov, Andrey V.; Campion, Richard P.; Kent, Anthony J.
2015-01-01
Phonon optics concerns operations with high-frequency acoustic waves in solid media in a similar way to how traditional optics operates with the light beams (i.e. photons). Phonon optics experiments with coherent terahertz and sub-terahertz phonons promise a revolution in various technical applications related to high-frequency acoustics, imaging, and heat transport. Previously, phonon optics used passive methods for manipulations with propagating phonon beams that did not enable their external control. Here we fabricate a phononic chip, which includes a generator of coherent monochromatic phonons with frequency 378 GHz, a sensitive coherent phonon detector, and an active layer: a doped semiconductor superlattice, with electrical contacts, inserted into the phonon propagation path. In the experiments, we demonstrate the modulation of the coherent phonon flux by an external electrical bias applied to the active layer. Phonon optics using external control broadens the spectrum of prospective applications of phononics on the nanometer scale. PMID:25652241
Engineering dissipation with phononic spectral hole burning.
Behunin, R O; Kharel, P; Renninger, W H; Rakich, P T
2017-03-01
Optomechanics, nano-electromechanics, and integrated photonics have brought about a renaissance in phononic device physics and technology. Central to this advance are devices and materials supporting ultra-long-lived photonic and phononic excitations that enable novel regimes of classical and quantum dynamics based on tailorable photon-phonon coupling. Silica-based devices have been at the forefront of such innovations for their ability to support optical excitations persisting for nearly 1 billion cycles, and for their low optical nonlinearity. While acoustic phonon modes can persist for a similar number of cycles in crystalline solids at cryogenic temperatures, it has not been possible to achieve such performance in silica, as silica becomes acoustically opaque at low temperatures. We demonstrate that these intrinsic forms of phonon dissipation are greatly reduced (by >90%) by nonlinear saturation using continuous drive fields of disparate frequencies. The result is a form of steady-state phononic spectral hole burning that produces a wideband transparency window with optically generated phonon fields of modest (nW) powers. We developed a simple model that explains both dissipative and dispersive changes produced by phononic saturation. Our studies, conducted in a microscale device, represent an important step towards engineerable phonon dynamics on demand and the use of glasses as low-loss phononic media.
Engineering dissipation with phononic spectral hole burning
NASA Astrophysics Data System (ADS)
Behunin, R. O.; Kharel, P.; Renninger, W. H.; Rakich, P. T.
2016-12-01
Optomechanics, nano-electromechanics, and integrated photonics have brought about a renaissance in phononic device physics and technology. Central to this advance are devices and materials supporting ultra-long-lived photonic and phononic excitations that enable novel regimes of classical and quantum dynamics based on tailorable photon-phonon coupling. Silica-based devices have been at the forefront of such innovations for their ability to support optical excitations persisting for nearly 1 billion cycles, and for their low optical nonlinearity. While acoustic phonon modes can persist for a similar number of cycles in crystalline solids at cryogenic temperatures, it has not been possible to achieve such performance in silica, as silica becomes acoustically opaque at low temperatures. We demonstrate that these intrinsic forms of phonon dissipation are greatly reduced (by >90%) by nonlinear saturation using continuous drive fields of disparate frequencies. The result is a form of steady-state phononic spectral hole burning that produces a wideband transparency window with optically generated phonon fields of modest (nW) powers. We developed a simple model that explains both dissipative and dispersive changes produced by phononic saturation. Our studies, conducted in a microscale device, represent an important step towards engineerable phonon dynamics on demand and the use of glasses as low-loss phononic media.
Spontaneous sidebanding in high speed rotordynamics
NASA Astrophysics Data System (ADS)
Ehrich, F. F.
1992-10-01
It is noted that the spontaneous sideband spacing frequency seems to be a whole number fraction (1/J) of the operating speed which indicates that the wave form is periodic and completes a full cycle every J rotations of the rotor. Employing a numerical model of a rotor that simulates local contact with a stator in close proximity as a bilinear spring, studies have been conducted to explore the circumstances for this spontaneous sidebanding. Two general classes of this type of response are determined in a system that is effectively single-degree-of-freedom.
Single sideband communications. Citations from the NTIS data base
NASA Astrophysics Data System (ADS)
Reed, W. E.
1980-08-01
Federally sponsored research on single sideband communication equipment and systems is presented. Reports on the design, development, and operation are cited. Studies on single sideband transmission, modulation, and single processing are included.
Optical pulse synthesis using brillouin selective sideband amplification
NASA Technical Reports Server (NTRS)
Yao, X. Steve (Inventor)
2002-01-01
Techniques for producing optical pulses based on Brillouin selective sideband amplification by using a common modulation control signal to modulate both a signal beam to produce multiple sideband signals and a single pump beam to produce multiple pump beams.
Second Harmonic Generation of Nanoscale Phonon Wave Packets.
Bojahr, A; Gohlke, M; Leitenberger, W; Pudell, J; Reinhardt, M; von Reppert, A; Roessle, M; Sander, M; Gaal, P; Bargheer, M
2015-11-06
Phonons are often regarded as delocalized quasiparticles with certain energy and momentum. The anharmonic interaction of phonons determines macroscopic properties of the solid, such as thermal expansion or thermal conductivity, and a detailed understanding becomes increasingly important for functional nanostructures. Although phonon-phonon scattering processes depicted in simple wave-vector diagrams are the basis of theories describing these macroscopic phenomena, experiments directly accessing these coupling channels are scarce. We synthesize monochromatic acoustic phonon wave packets with only a few cycles to introduce nonlinear phononics as the acoustic counterpart to nonlinear optics. Control of the wave vector, bandwidth, and consequently spatial extent of the phonon wave packets allows us to observe nonlinear phonon interaction, in particular, second harmonic generation, in real time by wave-vector-sensitive Brillouin scattering with x-rays and optical photons.
Motional sideband excitation using rotating electric fields
NASA Astrophysics Data System (ADS)
Isaac, C. A.
2013-04-01
A form of motional sideband excitation is described in which a rotating dipole electric field is applied asymmetrically onto a Penning-type trap in the presence of a mechanism for cooling the axial motion of the trapped particles. In contrast to the traditional motional sideband excitation, which uses an oscillating electric field, the rotating field results in only one active sideband in each sense of rotation and so avoids accidental excitation of the other sideband making it applicable to Penning-type traps with a large degree of anharmonicity. Expressions are derived for the magnetron radius expansion and compression rates attainable, and approximations are made for the case of strong and weak drives. A comparison is made with data, taken using a two-stage positron accumulator presented by Isaac [C. A. Isaac, C. J. Baker, T. Mortensen, D. P. van der Werf, and M. Charlton, Phys. Rev. Lett.PRLTAO0031-900710.1103/PhysRevLett.107.033201 107, 033201 (2011)], showing good agreement between the model and experiment.
Wide-Stopband Aperiodic Phononic Filters
NASA Technical Reports Server (NTRS)
Rostem, Karwan; Chuss, David; Denis, K. L.; Wollack, E. J.
2016-01-01
We demonstrate that a phonon stopband can be synthesized from an aperiodic structure comprising a discrete set of phononic filter stages. Each element of the set has a dispersion relation that defines a complete bandgap when calculated under a Bloch boundary condition. Hence, the effective stopband width in an aperiodic phononic filter (PnF) may readily exceed that of a phononic crystal with a single lattice constant or a coherence scale. With simulations of multi-moded phononic waveguides, we discuss the effects of finite geometry and mode-converting junctions on the phonon transmission in PnFs. The principles described may be utilized to form a wide stopband in acoustic and surface wave media. Relative to the quantum of thermal conductance for a uniform mesoscopic beam, a PnF with a stopband covering 1.6-10.4 GHz is estimated to reduce the thermal conductance by an order of magnitude at 75 mK.
Sideband cooling beyond the quantum backaction limit with squeezed light
NASA Astrophysics Data System (ADS)
Clark, Jeremy B.; Lecocq, Florent; Simmonds, Raymond W.; Aumentado, José; Teufel, John D.
2017-01-01
Quantum fluctuations of the electromagnetic vacuum produce measurable physical effects such as Casimir forces and the Lamb shift. They also impose an observable limit—known as the quantum backaction limit—on the lowest temperatures that can be reached using conventional laser cooling techniques. As laser cooling experiments continue to bring massive mechanical systems to unprecedentedly low temperatures, this seemingly fundamental limit is increasingly important in the laboratory. Fortunately, vacuum fluctuations are not immutable and can be ‘squeezed’, reducing amplitude fluctuations at the expense of phase fluctuations. Here we propose and experimentally demonstrate that squeezed light can be used to cool the motion of a macroscopic mechanical object below the quantum backaction limit. We first cool a microwave cavity optomechanical system using a coherent state of light to within 15 per cent of this limit. We then cool the system to more than two decibels below the quantum backaction limit using a squeezed microwave field generated by a Josephson parametric amplifier. From heterodyne spectroscopy of the mechanical sidebands, we measure a minimum thermal occupancy of 0.19 ± 0.01 phonons. With our technique, even low-frequency mechanical oscillators can in principle be cooled arbitrarily close to the motional ground state, enabling the exploration of quantum physics in larger, more massive systems.
ERIC Educational Resources Information Center
Beyer, Robert
1981-01-01
Surveys 50 years of acoustical studies by discussing selected topics including the ear, nonlinear representations, underwater sound, acoustical diagnostics, absorption, electrolytes, phonons, magnetic interaction, and superfluidity and the five sounds. (JN)
Terahertz-sideband spectra involving Kapteyn series
NASA Astrophysics Data System (ADS)
Lerche, Ian; Tautz, Robert C.; Citrin, D. S.
2009-09-01
Kapteyn series of the second kind appear in models of even- and odd-order sideband spectra in the optical regime of a quantum system modulated by a high-frequency (e.g., terahertz) electromagnetic field (Citrin D S 1999 Phys. Rev. B 60 5659) and in certain time-periodic transport problems in superlattices (Ignatov A A and Romanov Y A 1976 Phys. Status Solidi b 73 327; Feise M W and Citrin D S 1999 Appl. Phys. Lett. 75 3536). This paper shows that both the even- and the odd-order Kapteyn series that appear can be summed in closed form, thereby allowing more transparent insight into the structural dependence of the sideband spectra and also providing an analytic control for the accuracy of numerical procedures designed to evaluate the series. The general method of analysis may also be of interest for other Kapteyn series.
NASA Astrophysics Data System (ADS)
Yu, Si-Yuan; Sun, Xiao-Chen; Ni, Xu; Wang, Qing; Yan, Xue-Jun; He, Cheng; Liu, Xiao-Ping; Feng, Liang; Lu, Ming-Hui; Chen, Yan-Feng
2016-12-01
Strategic manipulation of wave and particle transport in various media is the key driving force for modern information processing and communication. In a strongly scattering medium, waves and particles exhibit versatile transport characteristics such as localization, tunnelling with exponential decay, ballistic, and diffusion behaviours due to dynamical multiple scattering from strong scatters or impurities. Recent investigations of graphene have offered a unique approach, from a quantum point of view, to design the dispersion of electrons on demand, enabling relativistic massless Dirac quasiparticles, and thus inducing low-loss transport either ballistically or diffusively. Here, we report an experimental demonstration of an artificial phononic graphene tailored for surface phonons on a LiNbO3 integrated platform. The system exhibits Dirac quasiparticle-like transport, that is, pseudo-diffusion at the Dirac point, which gives rise to a thickness-independent temporal beating for transmitted pulses, an analogue of Zitterbewegung effects. The demonstrated fully integrated artificial phononic graphene platform here constitutes a step towards on-chip quantum simulators of graphene and unique monolithic electro-acoustic integrated circuits.
Yu, Si-Yuan; Sun, Xiao-Chen; Ni, Xu; Wang, Qing; Yan, Xue-Jun; He, Cheng; Liu, Xiao-Ping; Feng, Liang; Lu, Ming-Hui; Chen, Yan-Feng
2016-12-01
Strategic manipulation of wave and particle transport in various media is the key driving force for modern information processing and communication. In a strongly scattering medium, waves and particles exhibit versatile transport characteristics such as localization, tunnelling with exponential decay, ballistic, and diffusion behaviours due to dynamical multiple scattering from strong scatters or impurities. Recent investigations of graphene have offered a unique approach, from a quantum point of view, to design the dispersion of electrons on demand, enabling relativistic massless Dirac quasiparticles, and thus inducing low-loss transport either ballistically or diffusively. Here, we report an experimental demonstration of an artificial phononic graphene tailored for surface phonons on a LiNbO3 integrated platform. The system exhibits Dirac quasiparticle-like transport, that is, pseudo-diffusion at the Dirac point, which gives rise to a thickness-independent temporal beating for transmitted pulses, an analogue of Zitterbewegung effects. The demonstrated fully integrated artificial phononic graphene platform here constitutes a step towards on-chip quantum simulators of graphene and unique monolithic electro-acoustic integrated circuits.
NASA Technical Reports Server (NTRS)
Goodman, Jerry R.; Grosveld, Ferdinand
2007-01-01
The acoustics environment in space operations is important to maintain at manageable levels so that the crewperson can remain safe, functional, effective, and reasonably comfortable. High acoustic levels can produce temporary or permanent hearing loss, or cause other physiological symptoms such as auditory pain, headaches, discomfort, strain in the vocal cords, or fatigue. Noise is defined as undesirable sound. Excessive noise may result in psychological effects such as irritability, inability to concentrate, decrease in productivity, annoyance, errors in judgment, and distraction. A noisy environment can also result in the inability to sleep, or sleep well. Elevated noise levels can affect the ability to communicate, understand what is being said, hear what is going on in the environment, degrade crew performance and operations, and create habitability concerns. Superfluous noise emissions can also create the inability to hear alarms or other important auditory cues such as an equipment malfunctioning. Recent space flight experience, evaluations of the requirements in crew habitable areas, and lessons learned (Goodman 2003; Allen and Goodman 2003; Pilkinton 2003; Grosveld et al. 2003) show the importance of maintaining an acceptable acoustics environment. This is best accomplished by having a high-quality set of limits/requirements early in the program, the "designing in" of acoustics in the development of hardware and systems, and by monitoring, testing and verifying the levels to ensure that they are acceptable.
Three material and four material one-dimensional phononic crystals
NASA Astrophysics Data System (ADS)
Kriegel, Ilka; Scotognella, Francesco
2017-01-01
In this work, we studied one-dimensional phononic structures for selective acoustic filtering. The structures are composed of three and four materials which have different elastic properties. We have observed that the phononic band gaps split in two and three transmission valleys for the three-material and the four-material based phononic structures, respectively. Furthermore, the number of transmission peaks between the split gaps is directly related to the number of unit cells composing the phononic structures. The observations of this work can be useful for the fabrication of acoustic filters with the possibility to select the transmission of particular frequencies.
Engineering interactions between superconducting qubits and phononic nanostructures
NASA Astrophysics Data System (ADS)
Arrangoiz-Arriola, Patricio; Safavi-Naeini, Amir H.
2016-12-01
Nanomechanical systems can support highly coherent microwave-frequency excitations at cryogenic temperatures. However, generating sufficient coupling between these devices and superconducting quantum circuits is challenging due to the vastly different length scales of acoustic and electromagnetic excitations. Here we demonstrate a general method for calculating piezoelectric interactions between quantum circuits and arbitrary phononic nanostructures. We illustrate our technique by studying the coupling between a transmon qubit and bulk acoustic-wave, Lamb-wave, and phononic crystal resonators, and show that very large coupling rates are possible in all three cases. Our results suggest a route to phononic circuits and systems that are nonlinear at the single-phonon level.
Phonon Analysis in Multiphonon Transitions
NASA Astrophysics Data System (ADS)
Huang, Kun; Gu, Zongquan
In the investigation of multiphonon transitions, single-mode or single-frequency models are widely used. In view of the fact that such oversimplified models can be seriously inadequate, the present work bridges the gap between the complexity of the general formal theory and the simplicity required for concrete applications by introducing the concept of multi-frequency models. That is, the theory is so formulated that a general system can be approximated by multi-frequency models of any degree of elaboration. A statistical thermodynamic formalism is developed for treating such multi-frequency models, which, on the one hand, greatly reduces the labour of calculation with such models and, on the other hand, leads directly to a simple statistical distribution law for numbers of phonons of each frequency participating in a multiphonon transition. Applications of the theory to concrete models lead to certain general conclusions on frequency dispersion effects in multiphonon transitions. The use of the theory is further demonstrated by fully accounting for the paradoxical experimental results reported by Jia and Yen that the isotopic substitution of H by D in CsMn Cl3· 2H2O reduces the multiphonon nonradiative transition probability of excited Mn2+ ion by more than ten-fold, and yet leaves the corresponding luminescence phonon sideband little changed. In the last section of the paper, the relation between the statistical thermodynamic formalism and existing multiphonon transition theory is elucidated, thereby the theoretical basis of the statistical formalism becomes clearly defined.
Hypersonic phonon propagation in one-dimensional surface phononic crystal
NASA Astrophysics Data System (ADS)
Graczykowski, B.; Sledzinska, M.; Kehagias, N.; Alzina, F.; Reparaz, J. S.; Sotomayor Torres, C. M.
2014-03-01
Hypersonic, thermally activated surface acoustic waves propagating in the surface of crystalline silicon patterned with periodic stripes were studied by Brillouin light scattering. Two characteristic directions (normal and parallel to the stripes) of surface acoustic waves propagation were examined exhibiting a distinctive propagation behavior. The measured phononic band structure exhibits diverse features, such as zone folding, band gap opening, and hybridization to local resonance for waves propagating normal to the stripes, and a variety of dispersive modes propagating along the stripes. Experimental results were supported by theoretical calculations performed using finite element method.
Phonon manipulation with phononic crystals.
Kim Bongsang; Hopkins, Patrick Edward; Leseman, Zayd C.; Goettler, Drew F.; Su, Mehmet F.; El-Kady, Ihab Fathy; Reinke, Charles M.; Olsson, Roy H., III
2012-01-01
In this work, we demonstrated engineered modification of propagation of thermal phonons, i.e. at THz frequencies, using phononic crystals. This work combined theoretical work at Sandia National Laboratories, the University of New Mexico, the University of Colorado Boulder, and Carnegie Mellon University; the MESA fabrication facilities at Sandia; and the microfabrication facilities at UNM to produce world-leading control of phonon propagation in silicon at frequencies up to 3 THz. These efforts culminated in a dramatic reduction in the thermal conductivity of silicon using phononic crystals by a factor of almost 30 as compared with the bulk value, and about 6 as compared with an unpatterned slab of the same thickness. This work represents a revolutionary advance in the engineering of thermoelectric materials for optimal, high-ZT performance. We have demonstrated the significant reduction of the thermal conductivity of silicon using phononic crystal structuring using MEMS-compatible fabrication techniques and in a planar platform that is amenable to integration with typical microelectronic systems. The measured reduction in thermal conductivity as compared to bulk silicon was about a factor of 20 in the cross-plane direction [26], and a factor of 6 in the in-plane direction. Since the electrical conductivity was only reduced by a corresponding factor of about 3 due to the removal of conductive material (i.e., porosity), and the Seebeck coefficient should remain constant as an intrinsic material property, this corresponds to an effective enhancement in ZT by a factor of 2. Given the number of papers in literature devoted to only a small, incremental change in ZT, the ability to boost the ZT of a material by a factor of 2 simply by reducing thermal conductivity is groundbreaking. The results in this work were obtained using silicon, a material that has benefitted from enormous interest in the microelectronics industry and that has a fairly large thermoelectric power
Yi, Kyung-Soo; Kim, Hye-Jung
2017-02-15
We investigate spectral behavior of phonon spectral functions in an interacting multi-component hot carrier plasma. Spectral analysis of various phonon spectral functions is performed considering carrier-phonon channels of polar and nonpolar optical phonons, acoustic deformation-potential, and piezoelectric Coulomb couplings. Effects of phonon self-energy corrections are examined at finite temperature within a random phase approximation extended to include the effects of dynamic screening, plasmon-phonon coupling, and local-field corrections of the plasma species. We provide numerical data for the case of a photo-generated electron-hole plasma formed in a wurtzite GaN. Our result shows the clear significance of the multiplicity of the plasma species in the phonon spectral functions of a multi-component plasma giving rise to a variety of spectral behaviors of carrier-phonon coupled collective modes. A useful sum rule on the plasma-species-resolved dielectric functions is also found.
NASA Astrophysics Data System (ADS)
Yi, Kyung-Soo; Kim, Hye-Jung
2017-02-01
We investigate spectral behavior of phonon spectral functions in an interacting multi-component hot carrier plasma. Spectral analysis of various phonon spectral functions is performed considering carrier-phonon channels of polar and nonpolar optical phonons, acoustic deformation-potential, and piezoelectric Coulomb couplings. Effects of phonon self-energy corrections are examined at finite temperature within a random phase approximation extended to include the effects of dynamic screening, plasmon-phonon coupling, and local-field corrections of the plasma species. We provide numerical data for the case of a photo-generated electron-hole plasma formed in a wurtzite GaN. Our result shows the clear significance of the multiplicity of the plasma species in the phonon spectral functions of a multi-component plasma giving rise to a variety of spectral behaviors of carrier-phonon coupled collective modes. A useful sum rule on the plasma-species-resolved dielectric functions is also found.
Phononic crystals and elastodynamics: Some relevant points
Aravantinos-Zafiris, N.; Sigalas, M. M.; Kafesaki, M.; Economou, E. N.
2014-12-15
In the present paper we review briefly some of the first works on wave propagation in phononic crystals emphasizing the conditions for the creation of acoustic band-gaps and the role of resonances to the band-gap creation. We show that useful conclusions in the analysis of phononic band gap structures can be drawn by considering the mathematical similarities of the basic classical wave equation (Helmholtz equation) with Schrödinger equation and by employing basic solid state physics concepts and conclusions regarding electronic waves. In the second part of the paper we demonstrate the potential of phononic systems to be used as elastic metamaterials. This is done by demonstrating negative refraction in phononic crystals and subwavelength waveguiding in a linear chain of elastic inclusions, and by proposing a novel structure with close to pentamode behavior. Finally the potential of phononic structures to be used in liquid sensor applications is discussed and demonstrated.
Phononic crystals and elastodynamics: Some relevant points
NASA Astrophysics Data System (ADS)
Aravantinos-Zafiris, N.; Sigalas, M. M.; Kafesaki, M.; Economou, E. N.
2014-12-01
In the present paper we review briefly some of the first works on wave propagation in phononic crystals emphasizing the conditions for the creation of acoustic band-gaps and the role of resonances to the band-gap creation. We show that useful conclusions in the analysis of phononic band gap structures can be drawn by considering the mathematical similarities of the basic classical wave equation (Helmholtz equation) with Schrödinger equation and by employing basic solid state physics concepts and conclusions regarding electronic waves. In the second part of the paper we demonstrate the potential of phononic systems to be used as elastic metamaterials. This is done by demonstrating negative refraction in phononic crystals and subwavelength waveguiding in a linear chain of elastic inclusions, and by proposing a novel structure with close to pentamode behavior. Finally the potential of phononic structures to be used in liquid sensor applications is discussed and demonstrated.
Cavity sideband cooling of trapped molecules
Kowalewski, Markus; Vivie-Riedle, Regina de; Morigi, Giovanna; Pinkse, Pepijn W. H.
2011-09-15
The efficiency of cavity sideband cooling of trapped molecules is theoretically investigated for the case in which the infrared transition between two rovibrational states is used as a cycling transition. The molecules are assumed to be trapped either by a radiofrequency or optical trapping potential, depending on whether they are charged or neutral, and confined inside a high-finesse optical resonator that enhances radiative emission into the cavity mode. Using realistic experimental parameters and COS as a representative molecular example, we show that in this setup, cooling to the trap ground state is feasible.
Phonons and elasticity of cementite through the Curie temperature
NASA Astrophysics Data System (ADS)
Mauger, L.; Herriman, J. E.; Hellman, O.; Tracy, S. J.; Lucas, M. S.; Muñoz, J. A.; Xiao, Yuming; Li, J.; Fultz, B.
2017-01-01
Phonon partial densities of states (pDOS) of Fe573C were measured from cryogenic temperatures through the Curie transition at 460 K using nuclear resonant inelastic x-ray scattering. The cementite pDOS reveal that low-energy acoustic phonons shift to higher energies (stiffen) with temperature before the magnetic transition. This unexpected stiffening suggests strongly nonharmonic vibrational behavior that impacts the thermodynamics and elastic properties of cementite. Density functional theory calculations reproduced the anomalous stiffening observed experimentally in cementite by accounting for phonon-phonon interactions at finite temperatures. The calculations show that the low-energy acoustic phonon branches with polarizations along the [010] direction are largely responsible for the anomalous thermal stiffening. The effect was further localized to the motions of the FeII site within the orthorhombic structure, which participates disproportionately in the anomalous phonon stiffening.
Transmission performance of the double-sideband SCM optical label
NASA Astrophysics Data System (ADS)
Chen, Minghua; Zhou, Weiqing; Jia, Zhensheng; Xie, Shizhong
2002-09-01
Transmission performance of the optical label with the double-sideband subcarrier multiplexing is investigated using Volterra transfer function approach. It is shown that the phase shifts of the two sideband signal is induced jointly by the interaction between SCM component and payload component due to fiber dispersion and nonlinearity. This will cause the SCM label fading, and then harm to system performance.
El-Kady, Ihab F [Albuquerque, NM; Olsson, Roy H [Albuquerque, NM
2012-01-10
Phononic crystals that have the ability to modify and control the thermal black body phonon distribution and the phonon component of heat transport in a solid. In particular, the thermal conductivity and heat capacity can be modified by altering the phonon density of states in a phononic crystal. The present invention is directed to phononic crystal devices and materials such as radio frequency (RF) tags powered from ambient heat, dielectrics with extremely low thermal conductivity, thermoelectric materials with a higher ratio of electrical-to-thermal conductivity, materials with phononically engineered heat capacity, phononic crystal waveguides that enable accelerated cooling, and a variety of low temperature application devices.
Split-sideband spectroscopy in slowly modulated optomechanics
NASA Astrophysics Data System (ADS)
Aranas, E. B.; Fonseca, P. Z. G.; Barker, P. F.; Monteiro, T. S.
2016-11-01
Optomechanical coupling between the motion of a mechanical oscillator and a cavity represents a new arena for experimental investigation of quantum effects on the mesoscopic and macroscopic scale. The motional sidebands of the output of a cavity offer ultra-sensitive probes of the dynamics. We introduce a scheme whereby these sidebands split asymmetrically and show how they may be used as experimental diagnostics and signatures of quantum noise limited dynamics. We show split-sidebands with controllable asymmetry occur by simultaneously modulating the light-mechanical coupling g and the mechanical frequency, {ω }{{M}}—slowly and out-of-phase. Such modulations are generic but already occur in optically trapped set-ups where the equilibrium point of the oscillator is varied cyclically. We analyse recently observed, but overlooked, experimental split-sideband asymmetries; although not yet in the quantum regime, the data suggests that split sideband structures are easily accessible to future experiments.
Multiple Quantum Wells for P T -Symmetric Phononic Crystals
NASA Astrophysics Data System (ADS)
Poshakinskiy, A. V.; Poddubny, A. N.; Fainstein, A.
2016-11-01
We demonstrate that the parity-time symmetry for sound is realized in laser-pumped multiple-quantum-well structures. Breaking of the parity-time symmetry for the phonons with wave vectors corresponding to the Bragg condition makes the structure a highly selective acoustic wave amplifier. Single-mode distributed feedback phonon lasing is predicted for structures with realistic parameters.
Engineering a squeezed phonon reservoir with a bichromatic driving of a quantum dot
NASA Astrophysics Data System (ADS)
Gao, Bo; Li, Gao-xiang; Ficek, Zbigniew
2016-09-01
We demonstrate how an acoustic phonon bath when coupled to a quantum dot with the help of a bichromatic laser field may effectively form a quantum squeezed reservoir. This approach allows one to achieve an arbitrary degree of squeezing of the effective reservoir and it incorporates the properties of the reservoir into two parameters, which can be controlled by varying the ratio of the Rabi frequencies of the bichromatic field. It is found that for unequal Rabi frequencies, the effective reservoir may appear as a quantum squeezed field of ordinary or inverted harmonic oscillators. When the Rabi frequencies are equal the effective reservoir appears as a perfectly squeezed field in which the decay of one of the polarization quadratures of the quantum dot dipole moment is inhibited. The decay of the quantum dot to a stationary state which depends on the initial coherence is predicted. This unusual result is shown to be a consequence of a quantum-nondemolition-type coupling of the quantum dot to the engineered squeezed reservoir. The effect of the initial coherence on the steady-state dressed-state population distribution and the fluorescence spectrum is discussed in detail. The complete polarization of the dressed state population and asymmetric spectra composed of only a single Rabi sideband peak are obtained under strictly resonant excitation.
NASA Astrophysics Data System (ADS)
Sudhir, Vivishek; Wilson, Dalziel; Schilling, Ryan; Schuetz, Hendrik; Nunnenkamp, Andreas; Kippenberg, Tobias
Measurement-based feedback provides an avenue to study the delicate interplay between the quantum correlations established during the process of measurement, and their progressive obfuscation when exposed to uncorrelated noise in the form of fundamental quantum fluctuations in the feedback path. Here we demonstrate this tradeoff using a feedback strategy whose objective is to cool a nano-mechanical oscillator close to its ground state. The correlations established due to the measurement are revealed in the appearance of motional sideband asymmetry. The latter, faithfully measured using an optical heterodyne interferometer with an imprecision ~17 dB below that at the standard quantum limit, increases to 6% as the oscillator is feedback cooled to an occupation of 15 phonons. Further increase in the gain of the feedback loop leads to a decrease in the asymmetry. This is due to the addition of unavoidable quantum fluctuations in a feedback amplifier - photon shot-noise amplified by a homodyne detector in our case.
Xia, H. Patterson, R.; Feng, Y.; Shrestha, S.; Conibeer, G.
2014-08-11
The rates of charge carrier relaxation by phonon emission are of substantial importance in the field of hot carrier solar cell, primarily in investigation of mechanisms to slow down hot carrier cooling. In this work, energy and momentum resolved deformation potentials relevant to electron-phonon scattering are computed for wurtzite InN and GaN as well as an InN/GaN multiple quantum well (MQW) superlattice using ab-initio methods. These deformation potentials reveal important features such as discontinuities across the electronic bandgap of the materials and variations over tens of eV. The energy dependence of the deformation potential is found to be very similar for wurtzite nitrides despite differences between the In and Ga pseudopotentials and their corresponding electronic band structures. Charge carrier relaxation by this mechanism is expected to be minimal for electrons within a few eV of the conduction band edge. However, hole scattering at energies more accessible to excitation by solar radiation is possible between heavy and light hole states. Moderate reductions in overall scattering rates are observed in MQW relative to the bulk nitride materials.
Buijsse, Bart; van Laarhoven, Frank; Schmid, Andreas K.; Cambie, Rossana; Cabrini, Stefano; Jin, Jian; Glaeser, Robert M.
2011-01-01
A novel design is described for an aperture that blocks a half-plane of the electron diffraction pattern out to a desired scattering angle, and then – except for a narrow support beam – transmits all of the scattered electrons beyond that angle. Our proposed tulip-shaped design is thus a hybrid between the single-sideband (ssb) aperture, which blocks a full half-plane of the diffraction pattern, and the conventional (i.e. fully open) double-sideband (dsb) aperture. The benefits of this hybrid design include the fact that such an aperture allows one to obtain high-contrast images of weak-phase objects with the objective lens set to Scherzer defocus. We further demonstrate that such apertures can be fabricated from thin-foil materials by milling with a focused ion beam (FIB), and that such apertures are fully compatible with the requirements of imaging out to a resolution of at least 0.34 nm. As is known from earlier work with single-sideband apertures, however, the edge of such an aperture can introduce unwanted, electrostatic phase shifts due to charging. The principal requirement for using such an aperture in a routine data-collection mode is thus to discover appropriate materials, protocols for fabrication and processing, and conditions of use such that the hybrid aperture remains free of charging over long periods of time. PMID:22088443
Quantitative analysis of sideband coupling in photoinduced force microscopy
NASA Astrophysics Data System (ADS)
Jahng, Junghoon; Kim, Bongsu; Lee, Eun Seong; Potma, Eric Olaf
2016-11-01
We present a theoretical and experimental analysis of the cantilever motions detected in photoinduced force microscopy (PiFM) using the sideband coupling detection scheme. In sideband coupling, the cantilever dynamics are probed at a combination frequency of a fundamental mechanical eigenmode and the modulation frequency of the laser beam. Using this detection mode, we develop a method for reconstructing the modulated photoinduced force gradient from experimental parameters in a quantitative manner. We show evidence, both theoretically and experimentally, that the sideband coupling detection mode provides PiFM images with superior contrast compared to images obtained when detecting the cantilever motions directly at the laser modulation frequency.
Thermal transport and anharmonic phonons in strained monolayer hexagonal boron nitride
Li, Shasha; Chen, Yue
2017-01-01
Thermal transport and phonon-phonon coupling in monolayer hexagonal boron nitride (h-BN) under equibiaxial strains are investigated from first principles. Phonon spectra at elevated temperatures have been calculated from perturbation theory using the third-order anharmonic force constants. The stiffening of the out-of-plane transverse acoustic mode (ZA) near the Brillouin zone center and the increase of acoustic phonon lifetimes are found to contribute to the dramatic increase of thermal transport in strained h-BN. The transverse optical mode (TO) at the K point, which was predicted to lead to mechanical failure of h-BN, is found to shift to lower frequencies at elevated temperatures under equibiaxial strains. The longitudinal and transverse acoustic modes exhibit broad phonon spectra under large strains in sharp contrast to the ZA mode, indicating strong in-plane phonon-phonon coupling. PMID:28262786
Thermal transport and anharmonic phonons in strained monolayer hexagonal boron nitride.
Li, Shasha; Chen, Yue
2017-03-06
Thermal transport and phonon-phonon coupling in monolayer hexagonal boron nitride (h-BN) under equibiaxial strains are investigated from first principles. Phonon spectra at elevated temperatures have been calculated from perturbation theory using the third-order anharmonic force constants. The stiffening of the out-of-plane transverse acoustic mode (ZA) near the Brillouin zone center and the increase of acoustic phonon lifetimes are found to contribute to the dramatic increase of thermal transport in strained h-BN. The transverse optical mode (TO) at the K point, which was predicted to lead to mechanical failure of h-BN, is found to shift to lower frequencies at elevated temperatures under equibiaxial strains. The longitudinal and transverse acoustic modes exhibit broad phonon spectra under large strains in sharp contrast to the ZA mode, indicating strong in-plane phonon-phonon coupling.
Thermal transport and anharmonic phonons in strained monolayer hexagonal boron nitride
NASA Astrophysics Data System (ADS)
Li, Shasha; Chen, Yue
2017-03-01
Thermal transport and phonon-phonon coupling in monolayer hexagonal boron nitride (h-BN) under equibiaxial strains are investigated from first principles. Phonon spectra at elevated temperatures have been calculated from perturbation theory using the third-order anharmonic force constants. The stiffening of the out-of-plane transverse acoustic mode (ZA) near the Brillouin zone center and the increase of acoustic phonon lifetimes are found to contribute to the dramatic increase of thermal transport in strained h-BN. The transverse optical mode (TO) at the K point, which was predicted to lead to mechanical failure of h-BN, is found to shift to lower frequencies at elevated temperatures under equibiaxial strains. The longitudinal and transverse acoustic modes exhibit broad phonon spectra under large strains in sharp contrast to the ZA mode, indicating strong in-plane phonon-phonon coupling.
Toward stimulated interaction of surface phonon polaritons
Kong, B. D.; Trew, R. J.; Kim, K. W.
2013-12-21
Thermal emission spectra mediated by surface phonon polariton are examined by using a theoretical model that accounts for generation processes. Specifically, the acoustic phonon fusion mechanism is introduced to remedy theoretical deficiencies of the near thermal equilibrium treatments. The model clarifies the thermal excitation mechanism of surface phonon polaritons and the energy transfer path under non-zero energy flow. When applied to GaAs and SiC semi-infinite surfaces, the nonequilibrium model predicts that the temperature dependence of the quasi-monochromatic peak can exhibit distinctly different characteristics of either sharp increase or slow saturation depending on the materials, which is in direct contrast with the estimate made by the near-equilibrium model. The proposed theoretical tool can accurately analyze the nonequilibrium steady states, potentially paving a pathway to demonstrate stimulated interaction/emission of thermally excited surface phonon polaritons.
Toward stimulated interaction of surface phonon polaritons
NASA Astrophysics Data System (ADS)
Kong, B. D.; Trew, R. J.; Kim, K. W.
2013-12-01
Thermal emission spectra mediated by surface phonon polariton are examined by using a theoretical model that accounts for generation processes. Specifically, the acoustic phonon fusion mechanism is introduced to remedy theoretical deficiencies of the near thermal equilibrium treatments. The model clarifies the thermal excitation mechanism of surface phonon polaritons and the energy transfer path under non-zero energy flow. When applied to GaAs and SiC semi-infinite surfaces, the nonequilibrium model predicts that the temperature dependence of the quasi-monochromatic peak can exhibit distinctly different characteristics of either sharp increase or slow saturation depending on the materials, which is in direct contrast with the estimate made by the near-equilibrium model. The proposed theoretical tool can accurately analyze the nonequilibrium steady states, potentially paving a pathway to demonstrate stimulated interaction/emission of thermally excited surface phonon polaritons.
Phononic crystals of poroelastic spheres
NASA Astrophysics Data System (ADS)
Alevizaki, A.; Sainidou, R.; Rembert, P.; Morvan, B.; Stefanou, N.
2016-11-01
An extension of the layer-multiple-scattering method to phononic crystals of poroelastic spheres immersed in a fluid medium is developed. The applicability of the method is demonstrated on specific examples of close-packed fcc crystals of submerged water-saturated meso- and macroporous silica microspheres. It is shown that, by varying the pore size and/or the porosity, the transmission, reflection, and absorption spectra of finite slabs of these crystals are significantly altered. Strong absorption, driven by the slow waves in the poroelastic material and enhanced by multiple scattering, leads to negligible transmittance over an extended frequency range, which might be useful for practical applications in broadband acoustic shielding. The results are analyzed by reference to relevant phononic dispersion diagrams in the viscous and inertial coupling limits, and a consistent interpretation of the underlying physics is provided.
Unexpectedly wide rf-induced synchrotron sideband depolarizing resonances
NASA Astrophysics Data System (ADS)
Chu, C. M.; Ellison, T. J.; Lee, S. Y.; Rinckel, T.; Schwandt, P.; Sperisen, F.; von Przewoski, B.; Anferov, V. A.; Blinov, B. B.; Bychkov, M. A.; Caussyn, D. D.; Courant, E. D.; Crandell, D. A.; Derbenev, Ya. S.; Kaufman, W. A.; Krisch, A. D.; Lorenzon, W.; Nurushev, T. S.; Phelps, R. A.; Ratner, L. G.; Wong, V. K.; Ohmori, C.; Minty, M. G.; Martin, P. S.; Russell, A. D.; Sivers, D. W.
1998-10-01
Using an rf solenoid magnet, we studied the depolarization of a stored 104.1 MeV vertically polarized proton beam. The two primary rf depolarizing resonances were properly centered around the protons' circulation frequency fc, at fc(3-νs) and fc(νs-1), where νs is the spin tune; moreover, each resonance was roughly consistent with the expected width of about 720 Hz. Each primary rf resonance had two synchrotron sideband resonances at the expected frequencies. The two νs-1 sidebands were deep dips while the two 3-νs sidebands were very shallow; this was not expected. Moreover, all four sideband resonances were unexpectedly wider than the two primary resonances.
Radiation pressure induced difference-sideband generation beyond linearized description
NASA Astrophysics Data System (ADS)
Xiong, Hao; Fan, Yu-Wan; Yang, Xiaoxue; Wu, Ying
2016-08-01
We investigate radiation-pressure induced generation of the frequency components at the difference-sideband in an optomechanical system, which beyond the conventional linearized description of optomechanical interactions between cavity fields and the mechanical oscillation. We analytically calculate amplitudes of these signals, and identify a simple square-root law for both the upper and lower difference-sideband generation which can describe the dependence of the intensities of these signals on the pump power. Further calculation shows that difference-sideband generation can be greatly enhanced via achieving the matching conditions. The effect of difference-sideband generation, which may have potential application for manipulation of light, is especially suited for on-chip optomechanical devices, where nonlinear optomechanical interaction in the weak coupling regime is within current experimental reach.
Optical frequency tripling with improved suppression and sideband selection.
Thakur, Manoj P; Medeiros, Maria C R; Laurêncio, Paula; Mitchell, John E
2011-12-12
A novel optical dispersion tolerant millimetre-wave radio-over-fibre system using optical frequency tripling technique with enhanced and selectable sideband suppression is demonstrated. The implementation utilises cascaded optical modulators to achieve either an optical single sideband (OSSB) or double sideband-suppressed carrier (DSB-SC) signal with high sideband suppression. Our analysis and simulation results indicate that the achievable suppression ratio of this configuration is only limited by other system factors such as optical noise and drifting of the operational conditions. The OSSB transmission system performance is assessed experimentally by the transport of 4 WiMax channels modulating a 10 GHz optical upconverted RF carrier as well as for optical frequency doubling and tripling. The 10 GHz and tripled carrier at 30 GHz are dispersion tolerant resulting both in an average relative constellation error (RCE) of -28.7 dB after 40 km of fibre.
Phononic Origins of Friction in Carbon Nanotube Oscillators.
Prasad, Matukumilli V D; Bhattacharya, Baidurya
2017-03-01
Phononic coupling can have a significant role in friction between nanoscale surfaces. We find frictional dissipation per atom in carbon nanotube (CNT) oscillators to depend significantly on interface features such as contact area, commensurability, and by end-capping of the inner core. We perform large-scale phonon wavepacket MD simulations to study phonon coupling between a 250 nm long (10,10) outer tube and inner cores of four different geometries. Five different phonon polarizations known to have dominant roles in thermal transport are selected, and transmission coefficient plots for a range of phonon energies along with phonon scattering dynamics at specific energies are obtained. We find that the length of interface affects friction only through LA phonon scattering and has a significant nonlinear effect on total frictional force. Incommensurate contact does not always give rise to superlubricity: the net effect of two competing interaction mechanisms shown by longitudinal and transverse phonons decides the role of commensurability. Capping of the core has no effect on acoustic phonons but destroys the coherence of transverse optical phonons and creates diffusive scattering. In contrast, the twisting and radial breathing phonon modes have perfect transmission at all energies and can be deemed as the enablers of ultralow friction in CNT oscillators. Our work suggests that tuning of interface geometries can give rise to desirable friction properties in nanoscale devices.
Derivation of sideband gain ratio for Herschel/HIFI
NASA Astrophysics Data System (ADS)
Kester, Do; Higgins, Ronan; Teyssier, David
2017-03-01
Context. Heterodyne mixers are commonly used for high-resolution spectroscopy at radio telescopes. When used as a double sideband system, the accurate flux calibration of spectral lines acquired by those detectors is highly dependent on the system gains in the respective mixer sidebands via the so-called sideband gain ratio (SBR). As such, the SBR was one of the main contributors to the calibration uncertainty budget of the Herschel/HIFI instrument. Aims: We want to determine the HIFI instrument sideband gain ratio for all bands on a fine frequency grid and within an accuracy of a few percent. Methods: We introduce a novel technique involving in-orbit HIFI data that is bootstrapped onto standard methods involving laboratory data measurements of the SBR. We deconvolved the astronomical data to provide a proxy of the expected signal at every frequency channel, and extracted the sideband gain ratios from the residuals of that process. Results: We determine the HIFI sideband gain ratio to an accuracy varying between 1 and 4%, with degraded accuracy in higher frequency ranges, and at places where the reliability of the technique is lower. These figures were incorporated into the HIFI data processing pipeline and improved the overall flux uncertainty of the legacy data from this instrument. Conclusions: We demonstrate that a modified sideband deconvolution algorithm, using astronomical data in combination with gas cell measurements, can be used to generate an accurate and fine-granularity picture of the sideband gain ratio behaviour of a heterodyne receiver. Herschel is an ESA space observatory with science instruments provided by European-led Principal Investigator consortia and with important participation from NASA.
Resolved Atomic Interaction Sidebands in an Optical Clock Transition
2011-06-24
Resolved Atomic Interaction Sidebands in an Optical Clock Transition M. Bishof,1 Y. Lin,1 M.D. Swallows,1 A.V. Gorshkov,2 J. Ye,1 and A.M. Rey1 1JILA...Institute of Technology, Pasadena, California 91125, USA (Received 4 February 2011; published 22 June 2011) We report the observation of resolved atomic ...interaction sidebands (ISB) in the 87Sr optical clock transition when atoms at microkelvin temperatures are confined in a two-dimensional optical lattice
Renormalisation of Nonequilibrium Phonons Under Strong Perturbative Influences.
NASA Astrophysics Data System (ADS)
Mehta, Sushrut Madhukar
Effects of strong perturbative influences, namely the presence of a narrow distribution of acoustic phonons, and the presence of an electron plasma, on the dynamics of nonequilibrium, near zone center, longitudinal optical phonons in GaP have been investigated in two separate experiments. The study of the effects of the interaction between the LO phonons and a heavily populated, narrow distribution of acoustic phonons lead to the observation of a new optically driven nonequilibrium phonon state. Time Resolved Coherent Antistokes Raman Scattering (TR-CARS), with picosecond resolution, was used to investigate the new mode. In order to achieve high occupation numbers in the acoustic branch, the picosecond laser pulses used were amplified up to 1.0 GW/cm^2 peak power per laser beam. An important characteristic property of the new state which differentiates it from the well known LO phonon state is the fact that rather than having the single decay rate observed under thermal equilibrium, the new state has two decay rates. Moreover, these two decay rates depend strongly on the distribution of the acoustic phonon occupation number. The coupling of the LO phonons with an electron plasma, on the other hand, was investigated by measurements of the shape of the Raman scattered line associated with the phonon-plasmon coupled mode. The plasma was generated by thermal excitation of carriers in doped samples. It was possible to study a large variety of plasma excitations by controlling the concentration of the dopant and the ambient temperature. A complete, self consistant model based on standard dielectric response theory is presented, and applied to the measurements of the phonon-plasmon coupled mode. It is possible to recover, via this model, the effective coupled mode damping rate, the plasma damping rate, and the plasma frequency as functions of ambient temperature, or the carrier concentration.
Manipulation of Phonons with Phononic Crystals
Leseman, Zayd Chad
2015-07-09
There were three research goals associated with this project. First, was to experimentally demonstrate phonon spectrum control at THz frequencies using Phononic Crystals (PnCs), i.e. demonstrate coherent phonon scattering with PnCs. Second, was to experimentally demonstrate analog PnC circuitry components at GHz frequencies. The final research goal was to gain a fundamental understanding of phonon interaction using computational methods. As a result of this work, 7 journal papers have been published, 1 patent awarded, 14 conference presentations given, 4 conference publications, and 2 poster presentations given.
Phonon Overlaps in Molecular Quantum Dot Systems
NASA Astrophysics Data System (ADS)
Chang, Connie; Sethna, James
2004-03-01
We model the amplitudes and frequencies of the vibrational sidebands for the new molecular quantum dot systems. We calculate the Franck-Condon phonon overlaps in the 3N-dimensional configuration sapce. We solve the general case where the vibrational frequencies and eigenmodes change during the transition. We perform PM3 and DFT calculations for the case of the dumb bell-shaped C140 molecule. We find that the strongest amplitudes are associated with the 11 meV stretch mode, in agreement with experiment. The experimental amplitudes vary from molecule to molecule; indicating that the molecular overlaps are environment dependent. We explore overlaps in the presence of external electric fields from image charges and counter ions.
Phonon Scattering Dynamics of Thermophoretic Motion in Carbon Nanotube Oscillators.
Prasad, Matukumilli V D; Bhattacharya, Baidurya
2016-04-13
Using phonon wave packet molecular dynamics simulations, we find that anomalous longitudinal acoustic (LA) mode phonon scattering in low to moderate energy ranges is responsible for initiating thermophoretic motion in carbon nanotube oscillators. The repeated scattering of a single mode LA phonon wave packet near the ends of the inner nanotube provides a net unbalanced force that, if large enough, initiates thermophoresis. By applying a coherent phonon pulse on the outer tube, which generalizes the single mode phonon wave packet, we are able to achieve thermophoresis in a carbon nanotube oscillator. We also find the nature of the unbalanced force on end-atoms to be qualitatively similar to that under an imposed thermal gradient. The thermodiffusion coefficient obtained for a range of thermal gradients and core lengths suggest that LA phonon scattering is the dominant mechanism for thermophoresis in longer cores, whereas for shorter cores, it is the highly diffusive mechanism that provides the effective force.
Phonon dynamics of graphene on metals
NASA Astrophysics Data System (ADS)
Taleb, Amjad Al; Farías, Daniel
2016-03-01
The study of surface phonon dispersion curves is motivated by the quest for a detailed understanding of the forces between the atoms at the surface and in the bulk. In the case of graphene, additional motivation comes from the fact that thermal conductivity is dominated by contributions from acoustic phonons, while optical phonon properties are essential to understand Raman spectra. In this article, we review recent progress made in the experimental determination of phonon dispersion curves of graphene grown on several single-crystal metal surfaces. The two main experimental techniques usually employed are high-resolution electron energy loss spectroscopy (HREELS) and inelastic helium atom scattering (HAS). The different dispersion branches provide a detailed insight into the graphene-substrate interaction. Softening of optical modes and signatures of the substrate‧s Rayleigh wave are observed for strong graphene-substrate interactions, while acoustic phonon modes resemble those of free-standing graphene for weakly interacting systems. The latter allows determining the bending rigidity and the graphene-substrate coupling strength. A comparison between theory and experiment is discussed for several illustrative examples. Perspectives for future experiments are discussed.
Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation.
Quilter, J H; Brash, A J; Liu, F; Glässl, M; Barth, A M; Axt, V M; Ramsay, A J; Skolnick, M S; Fox, A M
2015-04-03
We demonstrate a new method to realize the population inversion of a single InGaAs/GaAs quantum dot excited by a laser pulse tuned within the neutral exciton phonon sideband. In contrast to the conventional method of inverting a two-level system by performing coherent Rabi oscillation, the inversion is achieved by rapid thermalization of the optically dressed states via incoherent phonon-assisted relaxation. A maximum exciton population of 0.67±0.06 is measured for a laser tuned 0.83 meV to higher energy. Furthermore, the phonon sideband is mapped using a two-color pump-probe technique, with its spectral form and magnitude in very good agreement with the result of path-integral calculations.
Microscopic modeling of the effect of phonons on the optical properties of solid-state emitters
NASA Astrophysics Data System (ADS)
Norambuena, Ariel; Reyes, Sebastián A.; Mejía-Lopéz, José; Gali, Adam; Maze, Jerónimo R.
2016-10-01
Understanding the effect of vibrations in optically active nanosystems is crucial for successfully implementing applications in molecular-based electro-optical devices, quantum information communications, single photon sources, and fluorescent markers for biological measurements. Here, we present a first-principles microscopic description of the role of phonons on the isotopic shift presented in the optical emission spectrum associated to the negatively charged silicon-vacancy color center in diamond. We use the spin-boson model and estimate the electron-phonon interactions using a symmetrized molecular description of the electronic states and a force-constant model to describe molecular vibrations. Group theoretical arguments and dynamical symmetry breaking are presented in order to explain the optical properties of the zero-phonon line and the isotopic shift of the phonon sideband.
177-207 GHz Radiometer Front End: Single Sideband Measurements
NASA Technical Reports Server (NTRS)
Galin, I.; Schnitzer, C. A.; Dengler, R. J.; Quintero, O.
1999-01-01
Twenty years of progress in 200 GHz receivers for spaceborne remote sensing has yielded a 180-220 GHz technology with maturing characteristics, as evident by increasing availability of relevant hardware, paralleled by further refinement in receiver performance requirements at this spectrum band. The 177-207 GHz superheterodyne receiver, for the Earth observing system (EOS) microwave limb sounder (MLS), effectively illustrates such technology developments. This MLS receiver simultaneously detects six different signals, located at sidebands below and above its 191.95 GHZ local-oscillator (LO). The paper describes the MLS 177-207 GHz receiver front-end (RFE), and provides measured data for its lower and upper sidebands. Sideband ratio data is provided as a function of IF frequency, at different LO power drive, and for variation in the ambient temperature.
Methods and devices based on brillouin selective sideband amplification
NASA Technical Reports Server (NTRS)
Yao, X. Steve (Inventor)
2003-01-01
Opto-electronic devices and techniques using Brillouin scattering to select a sideband in a modulated optical carrier signal for amplification. Two lasers respectively provide a carrier signal beam and a Brillouin pump beam which are fed into an Brillouin optical medium in opposite directions. The relative frequency separation between the lasers is adjusted to align the frequency of the backscattered Brillouin signal with a desired sideband in the carrier signal to effect a Brillouin gain on the sideband. This effect can be used to implement photonic RF signal mixing and conversion with gain, conversion from phase modulation to amplitude modulation, photonic RF frequency multiplication, optical and RF pulse generation and manipulation, and frequency-locking of lasers.
Observation of wide rf induced synchrotron sideband depolarizing resonances.
NASA Astrophysics Data System (ADS)
Bychkov, M. A.; Anferov, V. A.; Blinov, B. B.; Courant, E. D.; Crandell, D. A.; Derbenev, Ya. S.; Kaufman, W. A.; Krisch, A. D.; Lorenzon, W.; Nurushev, T. S.; Phelps, R. A.; Wong, V. K.; Caussyn, D. D.; Chu, C. M.; Ellison, T. J. P.; Lee, S. Y.; Rinckel, T.; Schwandt, P.; Sperisen, F.; Stephenson, E. J.; von Przewoski, B.; Ohmori, C.; Minty, M. G.; Russell, A. D.
1997-04-01
In a recent experiment with a stored 104.1 MeV vertically polarized proton beam at the IUCF Cooler Ring, we depolarized the beam using an rf solenoid with a magnetic field of about 1.3\\cdot10-3T\\cdotm. We observed the two expected rf depolarizing resonances centered around the protons' 1.5 MHz circulation frequency as in previous experiments. Near each of these resonances, we also found synchrotron sidebands which are caused by the proton's energy oscillations. The strengths and widths of the synchrotron resonances were quite different for the sidebands above and below the circulation frequency.
Flexural-Phonon Scattering Induced by Electrostatic Gating in Graphene
NASA Astrophysics Data System (ADS)
Gunst, Tue; Kaasbjerg, Kristen; Brandbyge, Mads
2017-01-01
Graphene has an extremely high carrier mobility partly due to its planar mirror symmetry inhibiting scattering by the highly occupied acoustic flexural phonons. Electrostatic gating of a graphene device can break the planar mirror symmetry, yielding a coupling mechanism to the flexural phonons. We examine the effect of the gate-induced one-phonon scattering on the mobility for several gate geometries and dielectric environments using first-principles calculations based on density functional theory and the Boltzmann equation. We demonstrate that this scattering mechanism can be a mobility-limiting factor, and show how the carrier density and temperature scaling of the mobility depends on the electrostatic environment. Our findings may explain the high deformation potential for in-plane acoustic phonons extracted from experiments and, furthermore, suggest a direct relation between device symmetry and resulting mobility.
Iglesias, J. M.; Martín, M. J.; Pascual, E.; Rengel, R.
2016-01-25
We study, by means of a Monte Carlo simulator, the hot phonon effect on the relaxation dynamics in photoexcited graphene and its quantitative impact as compared with considering an equilibrium phonon distribution. Our multi-particle approach indicates that neglecting the hot phonon effect significantly underestimates the relaxation times in photoexcited graphene. The hot phonon effect is more important for a higher energy of the excitation pulse and photocarrier densities between 1 and 3 × 10{sup 12 }cm{sup −2}. Acoustic intervalley phonons play a non-negligible role, and emitted phonons with wavelengths limited up by a maximum (determined by the carrier concentration) induce a slower carrier cooling rate. Intrinsic phonon heating is damped in graphene on a substrate due to the additional cooling pathways, with the hot phonon effect showing a strong inverse dependence with the carrier density.
Sideband-controllable mode-locking fiber laser based on chirped fiber Bragg gratings.
Han, Dongdong; Liu, Xueming
2012-11-19
We have proposed a sideband-controllable fiber soliton laser by means of chirped fiber Bragg gratings (CFBGs). Each side of the spectral sidebands of laser could be removed by using a CFBG with proper dispersion. Numerical simulations have well reproduced the experimental observations. The numerical and experimental investigations show that the generation of the unilateral sidebands is attributed to the CFBG-induced spectral filtering effect. Our work provides an effective way to manage conventional solitons with spectral sidebands.
NASA Astrophysics Data System (ADS)
Nissimagoudar, A. S.; Sankeshwar, N. S.
2014-06-01
Lattice thermal conductivity, κp, of suspended and supported graphene nanoribbons (GNRs) is studied over a wide temperature range, taking into account the dispersive nature of confined acoustic phonon modes. Employing a modified Callaway model, an expression for κp is developed, considering the explicit contributions from in-plane longitudinal, transverse, and torsional acoustic, and out-of-plane flexural acoustic phonon modes. Numerical calculations of κp(T) are presented assuming the confined acoustic phonons to be scattered by sample boundaries, impurities, and other phonons via both normal and umklapp processes. The effect of phonon confinement is to modify the phonon group velocities and the temperature dependence of κp. In a suspended 5-nm-wide GNR at room temperature, a decrease in κp by ˜70% is predicted. Our study brings out the relative importance of the contributing phonon modes and reveals the influence of flexural phonons on κp as a marked shoulder at low temperatures. The role of the various sample-dependent scattering mechanisms is examined. The substrate, in supported GNRs, is shown to curtail the phonon mean free path and suppress the low-temperature κp. Our results are in good agreement with recent experimental data of Bae et al. [M. H. Bae, Z. Li, Z. Aksamija, P. N. Martin, F. Xiong, Z. Y. Ong, I. Knezevic, and E. Pop, Nat. Commun. 4, 1734 (2013), 10.1038/ncomms2755] for supported GNRs.
Phononic Frequency Comb via Intrinsic Three-Wave Mixing.
Ganesan, Adarsh; Do, Cuong; Seshia, Ashwin
2017-01-20
Optical frequency combs have resulted in significant advances in optical frequency metrology and found wide applications in precise physical measurements and molecular fingerprinting. A direct analogue of frequency combs in the phononic or acoustic domain has not been reported to date. In this Letter, we report the first clear experimental evidence for a phononic frequency comb. We show that the phononic frequency comb is generated through the intrinsic coupling of a driven phonon mode with an autoparametrically excited subharmonic mode. The experiments depict the comb generation process evidenced by a spectral response consisting of equally spaced discrete and phase coherent comb lines. Through systematic experiments at different drive frequencies and amplitudes, we portray the well-connected process of phononic frequency comb formation and define the attributes to control the features associated with comb formation in such a system. In addition to the demonstration of frequency comb, the interplay between the nonlinear resonances and the well-known Duffing phenomenon is also observed.
Phononic Frequency Comb via Intrinsic Three-Wave Mixing
NASA Astrophysics Data System (ADS)
Ganesan, Adarsh; Do, Cuong; Seshia, Ashwin
2017-01-01
Optical frequency combs have resulted in significant advances in optical frequency metrology and found wide applications in precise physical measurements and molecular fingerprinting. A direct analogue of frequency combs in the phononic or acoustic domain has not been reported to date. In this Letter, we report the first clear experimental evidence for a phononic frequency comb. We show that the phononic frequency comb is generated through the intrinsic coupling of a driven phonon mode with an autoparametrically excited subharmonic mode. The experiments depict the comb generation process evidenced by a spectral response consisting of equally spaced discrete and phase coherent comb lines. Through systematic experiments at different drive frequencies and amplitudes, we portray the well-connected process of phononic frequency comb formation and define the attributes to control the features associated with comb formation in such a system. In addition to the demonstration of frequency comb, the interplay between the nonlinear resonances and the well-known Duffing phenomenon is also observed.
NASA Astrophysics Data System (ADS)
Korkusinski, M.; Studenikin, S. A.; Aers, G.; Granger, G.; Kam, A.; Sachrajda, A. S.
2017-02-01
Manipulating qubits via electrical pulses in a piezoelectric material such as GaAs can be expected to generate incidental acoustic phonons. In this Letter we determine theoretically and experimentally the consequences of these phonons for semiconductor spin qubits using Landau-Zener-Stückelberg interferometry. Theoretical calculations predict that phonons in the presence of the spin-orbit interaction produce both phonon-Rabi fringes and accelerated evolution at the singlet-triplet anticrossing. Observed features confirm the influence of these mechanisms. Additionally, evidence is found that the pulsed gates themselves act as phonon cavities increasing the influence of phonons under specific resonant conditions.
Korkusinski, M; Studenikin, S A; Aers, G; Granger, G; Kam, A; Sachrajda, A S
2017-02-10
Manipulating qubits via electrical pulses in a piezoelectric material such as GaAs can be expected to generate incidental acoustic phonons. In this Letter we determine theoretically and experimentally the consequences of these phonons for semiconductor spin qubits using Landau-Zener-Stückelberg interferometry. Theoretical calculations predict that phonons in the presence of the spin-orbit interaction produce both phonon-Rabi fringes and accelerated evolution at the singlet-triplet anticrossing. Observed features confirm the influence of these mechanisms. Additionally, evidence is found that the pulsed gates themselves act as phonon cavities increasing the influence of phonons under specific resonant conditions.
Impact of resistive MHD plasma response on perturbation field sidebands
NASA Astrophysics Data System (ADS)
Orlov, D. M.; Evans, T. E.; Moyer, R. A.; Lyons, B. C.; Ferraro, N. M.; Park, G.-Y.
2016-07-01
Single fluid linear simulations of a KSTAR RMP ELM suppressed discharge with the M3D-C1 resistive magnetohydrodynamic code have been performed for the first time. The simulations show that the application of the n = 1 perturbation using the KSTAR in-vessel control coils (IVCC), which apply modest levels of n = 3 sidebands (~20% of the n = 1), leads to levels of n = 3 sideband that are comparable to the n = 1 when plasma response is included. This is due to the reduced level of screening of the rational-surface-resonant n = 3 component relative to the rational-surface-resonant n = 1 component. The n = 3 sidebands could play a similar role in ELM suppression on KSTAR as the toroidal sidebands (n = 1, 2, 4) in DIII-D n = 3 ELM suppression with missing I-coil segments (Paz Soldan et al 2014 Nucl. Fusion 54 073013). This result may help to explain the uniqueness of ELM suppression with n = 1 perturbations in KSTAR since the effective perturbation is a mixed n = 1/n = 3 perturbation similar to n = 3 ELM suppression in DIII-D.
Wang, Kai; Zhi, Miaochan; Hua, Xia; Sokolov, Alexei V
2014-09-08
Coherent Raman sidebands have the potential to serve as a source of single cycle pulses. We generate these sidebands by crossing two-color femtosecond laser pulses in a Raman-active crystal. We design a reflection scheme using spherical mirrors to combine coherent Raman sidebands. The sidebands and the driving pulses are refocused back to the Raman crystal and the relative spectral phases are retrieved from an interferogram based on the nonlinear Raman interaction. Furthermore, using a deformable mirror to adjust the spectral phases, we demonstrate that our setup is capable of synthesizing ultrafast waveforms using coherent Raman sidebands.
Optical studies of terahertz phonons dynamics in small-grain polycrystalline corundum
NASA Astrophysics Data System (ADS)
Feofilov, S. P.; Kaplyanskii, A. A.; Kulinkin, A. B.; Zakharchenya, R. I.
1999-03-01
The dynamics of terahertz acoustic phonons generated by optical pumping in ceramic-like α-Al 2O 3 with grain size ∼100 nm produced with the help of sol-gel technology was studied with the technique of optical detection of phonons by observation of probe Cr 3+ and Mn 4+ ions fluorescence. The dynamics of phonon distribution is very slow (∼ms) and drastically differs from that in regular α-Al 2O 3 ceramics with micron grain size and is similar to that observed earlier in oxide glasses. The results are discussed in the framework of studies of phonons in different structured and spatially restricted Al 2O 3 materials with different ratios between phonon wavelength λ and crystallite size a. It is shown that the acoustic mismatch model which describes phonon scattering in regular ceramics is not valid for small-grain sol-gel produced ceramics-like material.
Sideband characterization and atmospheric observations with various 340 GHz heterodyne receivers
NASA Astrophysics Data System (ADS)
Renker, Matthias; Murk, Axel; Rea, Simon P.; Emrich, A.; Frisk, U.
2014-08-01
This paper describes sideband response measurements and atmospheric observations with a double sideband and two Single Sideband (SSB) receiver prototypes developed for the multi-beam limb sounder instrument stratosphere-troposphere exchange and climate monitor radiometer. We first show an advanced Fourier-Transform Spectroscopy (FTS) method for sideband response and spurious signal characterization. We then present sideband response measurements of the different prototype receivers and we compare the results of the SSB receivers with sideband measurements by injecting a continuous wave signal into the upper and lower sidebands. The receivers were integrated into a total-power radiometer and atmospheric observations were carried out. The observed spectra were compared to forward model spectra to conclude on the sideband characteristics of the different receivers. The two sideband characterization methods show a high degree of agreement for both SSB receivers with various local oscillator settings. The measured sideband response was used to correct the forward model simulations. This improves the agreement with the atmospheric observations and explains spectral features caused by an unbalanced sideband response. The FTS method also allows to quantify the influence of spurious harmonic responses of the receiver.
Sideband characterization and atmospheric observations with various 340 GHz heterodyne receivers
Renker, Matthias Murk, Axel; Rea, Simon P.; Emrich, A.; Frisk, U.
2014-08-15
This paper describes sideband response measurements and atmospheric observations with a double sideband and two Single Sideband (SSB) receiver prototypes developed for the multi-beam limb sounder instrument stratosphere-troposphere exchange and climate monitor radiometer. We first show an advanced Fourier-Transform Spectroscopy (FTS) method for sideband response and spurious signal characterization. We then present sideband response measurements of the different prototype receivers and we compare the results of the SSB receivers with sideband measurements by injecting a continuous wave signal into the upper and lower sidebands. The receivers were integrated into a total-power radiometer and atmospheric observations were carried out. The observed spectra were compared to forward model spectra to conclude on the sideband characteristics of the different receivers. The two sideband characterization methods show a high degree of agreement for both SSB receivers with various local oscillator settings. The measured sideband response was used to correct the forward model simulations. This improves the agreement with the atmospheric observations and explains spectral features caused by an unbalanced sideband response. The FTS method also allows to quantify the influence of spurious harmonic responses of the receiver.
Phonon engineering for nanostructures.
Aubry, Sylvie; Friedmann, Thomas Aquinas; Sullivan, John Patrick; Peebles, Diane Elaine; Hurley, David H.; Shinde, Subhash L.; Piekos, Edward Stanley; Emerson, John Allen
2010-01-01
Understanding the physics of phonon transport at small length scales is increasingly important for basic research in nanoelectronics, optoelectronics, nanomechanics, and thermoelectrics. We conducted several studies to develop an understanding of phonon behavior in very small structures. This report describes the modeling, experimental, and fabrication activities used to explore phonon transport across and along material interfaces and through nanopatterned structures. Toward the understanding of phonon transport across interfaces, we computed the Kapitza conductance for {Sigma}29(001) and {Sigma}3(111) interfaces in silicon, fabricated the interfaces in single-crystal silicon substrates, and used picosecond laser pulses to image the thermal waves crossing the interfaces. Toward the understanding of phonon transport along interfaces, we designed and fabricated a unique differential test structure that can measure the proportion of specular to diffuse thermal phonon scattering from silicon surfaces. Phonon-scale simulation of the test ligaments, as well as continuum scale modeling of the complete experiment, confirmed its sensitivity to surface scattering. To further our understanding of phonon transport through nanostructures, we fabricated microscale-patterned structures in diamond thin films.
Coherent optical phonon oscillation and possible electronic softening in WTe2 crystals.
He, Bin; Zhang, Chunfeng; Zhu, Weida; Li, Yufeng; Liu, Shenghua; Zhu, Xiyu; Wu, Xuewei; Wang, Xiaoyong; Wen, Hai-Hu; Xiao, Min
2016-07-26
A rapidly-growing interest in WTe2 has been triggered by the giant magnetoresistance effect discovered in this unique system. While many efforts have been made towards uncovering the electron- and spin-relevant mechanisms, the role of lattice vibration remains poorly understood. Here, we study the coherent vibrational dynamics in WTe2 crystals by using ultrafast pump-probe spectroscopy. The oscillation signal in time domain in WTe2 has been ascribed as due to the coherent dynamics of the lowest energy A1 optical phonons with polarization- and wavelength-dependent measurements. With increasing temperature, the phonon energy decreases due to anharmonic decay of the optical phonons into acoustic phonons. Moreover, a significant drop (15%) of the phonon energy with increasing pump power is observed which is possibly caused by the lattice anharmonicity induced by electronic excitation and phonon-phonon interaction.
Coherent optical phonon oscillation and possible electronic softening in WTe2 crystals
He, Bin; Zhang, Chunfeng; Zhu, Weida; Li, Yufeng; Liu, Shenghua; Zhu, Xiyu; Wu, Xuewei; Wang, Xiaoyong; Wen, Hai-hu; Xiao, Min
2016-01-01
A rapidly-growing interest in WTe2 has been triggered by the giant magnetoresistance effect discovered in this unique system. While many efforts have been made towards uncovering the electron- and spin-relevant mechanisms, the role of lattice vibration remains poorly understood. Here, we study the coherent vibrational dynamics in WTe2 crystals by using ultrafast pump-probe spectroscopy. The oscillation signal in time domain in WTe2 has been ascribed as due to the coherent dynamics of the lowest energy A1 optical phonons with polarization- and wavelength-dependent measurements. With increasing temperature, the phonon energy decreases due to anharmonic decay of the optical phonons into acoustic phonons. Moreover, a significant drop (15%) of the phonon energy with increasing pump power is observed which is possibly caused by the lattice anharmonicity induced by electronic excitation and phonon-phonon interaction. PMID:27457385
Ultrafast optical generation of coherent phonons in CdTe1-xSex quantum dots
NASA Astrophysics Data System (ADS)
Bragas, A. V.; Aku-Leh, C.; Costantino, S.; Ingale, Alka; Zhao, J.; Merlin, R.
2004-05-01
We report on the impulsive generation of coherent optical phonons in CdTe0.68Se0.32 nanocrystallites embedded in a glass matrix. Pump-probe experiments using femtosecond laser pulses were performed by tuning the laser central energy to resonate with the absorption edge of the nanocrystals. We identify two longitudinal optical phonons, one longitudinal acoustic phonon and a fourth mode of a mixed longitudinal-transverse nature. The amplitude of the optical phonons as a function of the laser central energy exhibits a resonance that is well described by a model based on impulsive stimulated Raman scattering. The phases of the coherent phonons reveal coupling between different modes. At low power density excitations, the frequency of the optical coherent phonons deviates from values obtained from spontaneous Raman scattering. This behavior is ascribed to the presence of electronic impurity states which modify the nanocrystal dielectric function and, thereby, the frequency of the infrared-active phonons.
Strong acoustic coupling to a superconducting qubit
NASA Astrophysics Data System (ADS)
Gustafsson, Martin; Aref, Thomas; Frisk Kockum, Anton; Ekström, Maria; Johansson, Göran; Delsing, Per
2014-03-01
Micromechanical resonators can be used to store quantum information, as shown in several recent experiments. These resonators typically have the form of membranes or beams, and phonons are localized to their vibrational eigenmodes. We present a different kind of mechanical quantum device, where propagating phonons serve as carriers for quantum information. At the core of our device is a superconducting qubit, designed to couple to Surface Acoustic Waves (SAW) in the underlying substrate through the piezoelectric effect. This type of coupling can be very strong, and in our case exceeds the coupling to any external electromagnetic modes. The acoustic waves propagate freely on the surface of the substrate, and we use a remote electro-acoustic transducer to address the qubit acoustically and listen to its emission of phonons. This presentation focuses on the basic properties of our acoustic quantum system, and we include experimental data that demonstrate the quantized coupling between the qubit and the propagating acoustic waves.
Phonons in NaO/sub 2/ near the order-disorder transition
Wakabayashi, N.; Alefeld, B.; Buhrer, W.; Smith, H.G.
1982-10-15
The acoustic phonons in cubic NaO/sub 2/ have been studied above and below the order-disorder transition by inelastic neutron scattering. Above the transition the O/sub 2/ /sup -/ ions are disordered and undergoing rapid reorientation about the body diagonals. This reorientation couples with and affects certain acoustic modes in the crystal. The results are described in terms of a phonon-pseudospin coupling theory.
Research on micro-sized acoustic bandgap structures.
Fleming, James Grant; McCormick, Frederick Bossert; Su, Mehmet F.; El-Kady, Ihab Fathy; Olsson, Roy H., III; Tuck, Melanie R.
2010-01-01
Phononic crystals (or acoustic crystals) are the acoustic wave analogue of photonic crystals. Here a periodic array of scattering inclusions located in a homogeneous host material forbids certain ranges of acoustic frequencies from existence within the crystal, thus creating what are known as acoustic (or phononic) bandgaps. The vast majority of phononic crystal devices reported prior to this LDRD were constructed by hand assembling scattering inclusions in a lossy viscoelastic medium, predominantly air, water or epoxy, resulting in large structures limited to frequencies below 1 MHz. Under this LDRD, phononic crystals and devices were scaled to very (VHF: 30-300 MHz) and ultra (UHF: 300-3000 MHz) high frequencies utilizing finite difference time domain (FDTD) modeling, microfabrication and micromachining technologies. This LDRD developed key breakthroughs in the areas of micro-phononic crystals including physical origins of phononic crystals, advanced FDTD modeling and design techniques, material considerations, microfabrication processes, characterization methods and device structures. Micro-phononic crystal devices realized in low-loss solid materials were emphasized in this work due to their potential applications in radio frequency communications and acoustic imaging for medical ultrasound and nondestructive testing. The results of the advanced modeling, fabrication and integrated transducer designs were that this LDRD produced the 1st measured phononic crystals and phononic crystal devices (waveguides) operating in the VHF (67 MHz) and UHF (937 MHz) frequency bands and established Sandia as a world leader in the area of micro-phononic crystals.
Nanoscale interface engineering in ZnO twin nanorods for proposed phonon tunnel devices.
Singh, Avanendra; Senapati, Kartik; Satpati, Biswarup; Kumar, Mohit; Sahoo, Pratap K
2015-02-14
Zinc oxide twin nanorods, with two identical crystalline sections connected by an amorphous layer, were reproducibly grown using a simple one-step hydrothermal technique. The thickness of the amorphous layer between the crystalline segments was tunable with growth parameters, as confirmed by high resolution transmission electron microscopy. The photoluminescence spectra of these twin nanorods exhibit strong near band edge emission in the UV range, with convoluted phonon sidebands. De-convolution analyses of these spectra showed that the amorphous interlayers act as effective phonon barriers beyond a certain thickness. Such oriented grown individual crystalline-amorphous-crystalline structures may be a suitable test system for fundamental studies of phonon tunneling in the nanostructure. While physical vapor deposition techniques are seriously constrained in realizing crystalline-amorphous-crystalline structures, our results show the viability of engineering embedded interfaces via chemical routes.
Sideband growth in nonlinear Landau wave-particle interaction.
NASA Technical Reports Server (NTRS)
Brinca, A. L.
1972-01-01
The distortion of the electron velocity distribution caused by a large amplitude Landau wave is determined analytically for the initial-value problem. The resulting stability of electrostatic perturbations impressed on the evolving plasma is studied. Narrow sidebands of the applied frequency experience consecutive growths of large magnitude during the early stages of the nonlinear wave-particle interaction. The significance of the derived results to both wave propagation experiments and triggered VLF emissions in the magnetosphere is discussed.
Functional crossover in the dispersion relations of magnons and phonons
NASA Astrophysics Data System (ADS)
Hoser, A.; Köbler, U.
2016-09-01
Experimental data are presented showing that the dispersion relations of magnons and acoustic phonons can consist of two sections with different functions of wave vector. In the low wave vector range a power function of wave vector often holds over a finite q-range while dispersions for larger wave vector values better approach the atomistic model predictions. In the magnon spectra ∼⃒qx power functions with exponents x=1.25, 1.5 and 2 are identified. The dispersion of the acoustic phonons can be a linear function of wave vector over a surprisingly large range of energy. Since the slope of the linear section agrees with the known sound velocities it can be concluded that the dispersion of the acoustic phonons has got attracted by the linear dispersion of the mass less Debye bosons (sound waves). Due to the different (translational) symmetries of bosons and atomistic excitations (magnons, phonons) the associated dispersions can attract each other. In the same way the different ∼⃒qx power functions in the magnon dispersions indicate that magnon dispersions are attracted by the dispersion of the bosons of the magnetic continuum (Goldstone bosons). This allows evaluation of the otherwise difficult to obtain dispersions of the Goldstone bosons from the known magnon dispersions. Interestingly, the dispersions of Goldstone bosons (Debye bosons) attract magnon dispersions (phonon dispersions) and not vice versa.
Electron-phonon interaction model and prediction of thermal energy transport in SOI transistor.
Jin, Jae Sik; Lee, Joon Sik
2007-11-01
An electron-phonon interaction model is proposed and applied to thermal transport in semiconductors at micro/nanoscales. The high electron energy induced by the electric field in a transistor is transferred to the phonon system through electron-phonon interaction in the high field region of the transistor. Due to this fact, a hot spot occurs, which is much smaller than the phonon mean free path in the Si-layer. The full phonon dispersion model based on the Boltzmann transport equation (BTE) with the relaxation time approximation is applied for the interactions among different phonon branches and different phonon frequencies. The Joule heating by the electron-phonon scattering is modeled through the intervalley and intravalley processes for silicon by introducing average electron energy. The simulation results are compared with those obtained by the full phonon dispersion model which treats the electron-phonon scattering as a volumetric heat source. The comparison shows that the peak temperature in the hot spot region is considerably higher and more localized than the previous results. The thermal characteristics of each phonon mode are useful to explain the above phenomena. The optical mode phonons of negligible group velocity obtain the highest energy density from electrons, and resides in the hot spot region without any contribution to heat transport, which results in a higher temperature in that region. Since the acoustic phonons with low group velocity show the higher energy density after electron-phonon scattering, they induce more localized heating near the hot spot region. The ballistic features are strongly observed when phonon-phonon scattering rates are lower than 4 x 10(10) S(-1).
``Forbidden'' phonon in the iron chalcogenide series
NASA Astrophysics Data System (ADS)
Fobes, David M.; Zaliznyak, Igor A.; Xu, Zhijun; Gu, Genda; Tranquada, John M.
2015-03-01
Recently, we uncovered evidence for the formation of a bond-order wave (BOW) leading to ferro-orbital order at low temperature, acting to stabilize the bicollinear AFM order, in the iron-rich parent compound, Fe1+yTe. Investigating the inelastic spectra centered near (100) in Fe1+yTe, a signature peak for the BOW formation in the monoclinic phase, we observed an acoustic phonon dispersion in both tetragonal and monoclinic phases. While a structural Bragg peak accompanies the mode in the monoclinic phase, in the tetragonal phase Bragg scattering at this Q is forbidden by symmetry, and we observed no elastic peak. This phonon mode was also observed in superconducting FeTe0.6Se0.4, where structural and magnetic transitions are suppressed. LDA frozen phonon calculations suggested that this mode could result from a spin imbalance between neighboring Fe atoms, but polarized neutron measurements revealed no additional magnetic scattering. We propose that this ``forbidden'' phonon mode may originate from dynamically broken symmetry, perhaps related to the strong dynamic spin correlations in these materials. Work at BNL was supported by BES, US DOE, under Contract No. DE-AC02-98CH10886. Research at ORNL's HFIR and SNS sponsored by Scientific User Facilities Division, BES, US DOE. We acknowledge the support of NIST, in providing neutron research facilities.
Structure of crystalline oxide ceramics studied by phonon spectroscopy
Kaminskii, Alexandr A; Taranov, A V; Khazanov, E N
2013-03-31
This paper describes a method for gaining detailed insight into the structure and phonon spectrum of polycrystalline oxide ceramics. We examine how the diffusion coefficient of subterahertz phonons is related to the properties of a system of grain boundaries and to the grain size and structure and demonstrate that the temperature dependence of the phonon diffusion coefficient at liquid-helium temperatures is determined by the spectral properties of the intergranular layer, which allows one to estimate the volumeaveraged intergranular layer thickness and acoustic impedance. We also analyse the effect of plastic deformation via twinning on the formation of the structure of grains and intergranular layers, which determine the thermophysical, acoustic and optical properties of ceramic materials. (extreme light fields and their applications)
Molecular Detection and Phonon Filtering in Heat-Transfer Spectroscopy
NASA Astrophysics Data System (ADS)
Walczak, Kamil; Yerkes, Kirk
2014-03-01
We examine heat transport carried by acoustic phonons in the systems composed of nanoscale chains of masses coupled to two thermal baths of different temperatures. Thermal conductance is obtained by using linearized Landauer formula for heat flux with phonon transmission probability calculated within atomistic Green's functions (AGF) method. AGF formalism is extended onto dissipative chains of masses with harmonic coupling beyond nearest-neighbor approximation, while atomistic description of heat reservoirs is also included into computational scheme. The resonant structure of phonon transmission spectrum is analyzed with respect to reservoir-dimensionality effects, molecular damping, and mass-to-mass harmonic coupling. Analysis of transmission zeros (antiresonances) and their accompanied Fano-shape resonances are discussed as a result of interference effects between different vibrational modes. Specifically, we show that the heat-transfer-based characterization method may be used to identify individual molecules or filter out specific phonon modes from the whole frequency spectrum. This work is supported by AFOSR grant.
Wang, Wen Ting; Liu, Jian Guo; Mei, Hai Kuo; Zhu, Ning Hua
2016-01-11
We propose and experimentally verify a novel approach to achieve phase-coherence orthogonally polarized optical single sideband (OSSB) modulation with a tunable optically carrier-to-sideband ratio (OCSR). In our scheme, the orthogonally polarized OSSB signal is achieved using a dual-polarization quadrature phase shift keying (DP-QPSK) modulator without an optical band-pass filter (OBPF). Therefore, the proposed method is wavelength independent. The DP-QPSK modulator includes two parallel QPSK modulators locating on its two arms. The upper QPSK modulator of the DP-QPSK modulator is driven by two quadrature sinusoidal microwave signals and works at the frequency shifting condition whose bias voltages are optimized to suppress the optical. The lower QPSK modulator of that works at the maximum transmission point and the optical carrier is not modulated. The OCSR is continuously tunable by simply adjusting the bias voltages of the lower modulator. The frequency shifting optical signal from the upper QPSK modulator and the optical carrier from the lower QPSK modulator are combined together at the output of the DP-QPSK modulator. The optical carrier and sideband are polarized orthogonally. The generated OSSB signals could be used to shift and code the phase of the microwave signal and generate ultra-wideband (UWB) microwave pulse. The proposed method is analyzed and experimental demonstrated.
Temperature dependence of phonon-defect interactions: phonon scattering vs. phonon trapping
Bebek, M. B.; Stanley, C. M.; Gibbons, T. M.; Estreicher, S. K.
2016-01-01
The interactions between thermal phonons and defects are conventionally described as scattering processes, an idea proposed almost a century ago. In this contribution, ab-initio molecular-dynamics simulations provide atomic-level insight into the nature of these interactions. The defect is the Si|X interface in a nanowire containing a δ-layer (X is C or Ge). The phonon-defect interactions are temperature dependent and involve the trapping of phonons for meaningful lengths of time in defect-related, localized, vibrational modes. No phonon scattering occurs and the momentum of the phonons released by the defect is unrelated to the momentum of the phonons that generated the excitation. The results are extended to the interactions involving only bulk phonons and to phonon-defect interactions at high temperatures. These do resemble scattering since phonon trapping occurs for a length of time short enough for the momentum of the incoming phonon to be conserved. PMID:27535463
Phonon dispersion relation of metallic glasses
NASA Astrophysics Data System (ADS)
Crespo, Daniel; Bruna, Pere; Valles, Araceli; Pineda, Eloi
2016-10-01
Experimental data on the phase sound speed of metallic glasses show anomalies in the terahertz range, reflecting an underlying complex behavior of their phonon dispersion spectrum not yet explained. We determine the phonon dispersion curve of metallic glasses by means of massive molecular dynamics simulations, allowing us to obtain the low-q region behavior with unprecedented detail. Results confirm that the sound speed is constant below the THz range, down to the macroscopic limit. On the contrary, a hardening of the sound speed, more notable in the transverse case, is found in the THz range. This behavior is modeled in terms of a relaxation model. The model gives quantitative agreement and allows us to determine a new threshold frequency ωh, at the end of the boson-peak region. Above ωh the shear modulus increases dramatically, reflecting the end of the amorphous-like acoustic propagation region characterized by the excess density of vibrational states.
Tunable phonon-cavity coupling in graphene membranes
NASA Astrophysics Data System (ADS)
de Alba, R.; Massel, F.; Storch, I. R.; Abhilash, T. S.; Hui, A.; McEuen, P. L.; Craighead, H. G.; Parpia, J. M.
2016-09-01
A major achievement of the past decade has been the realization of macroscopic quantum systems by exploiting the interactions between optical cavities and mechanical resonators. In these systems, phonons are coherently annihilated or created in exchange for photons. Similar phenomena have recently been observed through phonon-cavity coupling—energy exchange between the modes of a single system mediated by intrinsic material nonlinearity. This has so far been demonstrated primarily for bulk crystalline, high-quality-factor (Q > 105) mechanical systems operated at cryogenic temperatures. Here, we propose graphene as an ideal candidate for the study of such nonlinear mechanics. The large elastic modulus of this material and capability for spatial symmetry breaking via electrostatic forces is expected to generate a wealth of nonlinear phenomena, including tunable intermodal coupling. We have fabricated circular graphene membranes and report strong phonon-cavity effects at room temperature, despite the modest Q factor (∼100) of this system. We observe both amplification into parametric instability (mechanical lasing) and the cooling of Brownian motion in the fundamental mode through excitation of cavity sidebands. Furthermore, we characterize the quenching of these parametric effects at large vibrational amplitudes, offering a window on the all-mechanical analogue of cavity optomechanics, where the observation of such effects has proven elusive.
Broadband evolution of phononic-crystal-waveguide eigenstates in real- and k-spaces.
Otsuka, P H; Nanri, K; Matsuda, O; Tomoda, M; Profunser, D M; Veres, I A; Danworaphong, S; Khelif, A; Benchabane, S; Laude, V; Wright, O B
2013-11-27
Control of sound in phononic band-gap structures promises novel control and guiding mechanisms. Designs in photonic systems were quickly matched in phononics, and rows of defects in phononic crystals were shown to guide sound waves effectively. The vast majority of work in such phononic guiding has been in the frequency domain, because of the importance of the phononic dispersion relation in governing acoustic confinement in waveguides. However, frequency-domain studies miss vital information concerning the phase of the acoustic field and eigenstate coupling. Using a wide range of wavevectors k, we implement an ultrafast technique to probe the wave field evolution in straight and L-shaped phononic crystal surface-phonon waveguides in real- and k-space in two spatial dimensions, thus revealing the eigenstate-energy redistribution processes and the coupling between different frequency-degenerate eigenstates. Such use of k-t space is a first in acoustics, and should have other interesting applications such as acoustic-metamaterial characterization.
NASA Astrophysics Data System (ADS)
Kuleev, I. I.; Bakharev, S. M.; Kuleev, I. G.; Ustinov, V. V.
2017-01-01
Effect of anisotropy of elastic energy on the phonon propagation in single-crystal nanowires made of Fe, Cu, MgO, InSb, and GaAs materials that are used to fabricate spintronics devices in the regime of the Knudsen flow of phonon gas has been studied. A new method of analyzing the focusing of quasi-transverse modes has been suggested, which made it possible to determine the average values of the densities of phonon states in the regions of focusing and defocusing slow and fast quasi-transverse modes. The effect of phonon focusing on the anisotropy of heat conductivity and lengths of the phonon free paths has been analyzed for all acoustic modes that exist in spintronics nanostructures. It has been shown that for all the nanowires investigated the angular dependences of the free paths of fast and slow transverse modes in the {100} and {110} planes correlate with the angular dependences of the densities of phonon states for these modes. Directions of the heat flux that ensure the maximum and minimum phonon heat conductivity in the nanowires have been determined.
Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2
Gardner, D. R.; Bonnoit, C. J.; Chisnell, R.; ...
2016-02-11
In this paper, we study high-resolution inelastic x-ray scattering measurements of the acoustic phonons of URu2Si2. At all temperatures, the longitudinal acoustic phonon linewidths are anomalously broad at small wave vectors revealing a previously unknown anharmonicity. The phonon modes do not change significantly upon cooling into the hidden order phase. In addition, our data suggest that the increase in thermal conductivity in the hidden order phase cannot be driven by a change in phonon dispersions or lifetimes. Hence, the phonon contribution to the thermal conductivity is likely much less significant compared to that of the magnetic excitations in the lowmore » temperature phase.« less
Coherent transfer of optical orbital angular momentum in multi-order Raman sideband generation.
Strohaber, J; Zhi, M; Sokolov, A V; Kolomenskii, A A; Paulus, G G; Schuessler, H A
2012-08-15
Experimental results from the generation of Raman sidebands using optical vortices are presented. By generating two sets of sidebands originating from different locations in a Raman-active crystal, one set containing optical orbital angular momentum and the other serving as a reference, Young's double slit experiment was simultaneously realized for each sideband. The interference between the two sets of sidebands was used to determine the helicity and topological charge in each order. Topological charges in all orders were found to be discrete and follow selection rules predicted by a cascaded Raman process.
First-principles prediction of phononic thermal conductivity of silicene: A comparison with graphene
Gu, Xiaokun; Yang, Ronggui
2015-01-14
There has been great interest in two-dimensional materials, beyond graphene, for both fundamental sciences and technological applications. Silicene, a silicon counterpart of graphene, has been shown to possess some better electronic properties than graphene. However, its thermal transport properties have not been fully studied. In this paper, we apply the first-principles-based phonon Boltzmann transport equation to investigate the thermal conductivity of silicene as well as the phonon scattering mechanisms. Although both graphene and silicene are two-dimensional crystals with similar crystal structure, we find that phonon transport in silicene is quite different from that in graphene. The thermal conductivity of silicene shows a logarithmic increase with respect to the sample size due to the small scattering rates of acoustic in-plane phonon modes, while that of graphene is finite. Detailed analysis of phonon scattering channels shows that the linear dispersion of the acoustic out-of-plane (ZA) phonon modes, which is induced by the buckled structure, makes the long-wavelength longitudinal acoustic phonon modes in silicene not as efficiently scattered as that in graphene. Compared with graphene, where most of the heat is carried by the acoustic out-of-plane (ZA) phonon modes, the ZA phonon modes in silicene only have ∼10% contribution to the total thermal conductivity, which can also be attributed to the buckled structure. This systematic comparison of phonon transport and thermal conductivity of silicene and graphene using the first-principle-based calculations shed some light on other two-dimensional materials, such as two-dimensional transition metal dichalcogenides.
Cavity sideband cooling of a single trapped ion.
Leibrandt, David R; Labaziewicz, Jaroslaw; Vuletić, Vladan; Chuang, Isaac L
2009-09-04
We report a demonstration and quantitative characterization of one-dimensional cavity cooling of a single trapped (88)Sr(+) ion in the resolved-sideband regime. We measure the spectrum of cavity transitions, the rates of cavity heating and cooling, and the steady-state cooling limit. The cavity cooling dynamics and cooling limit of 22.5(3) motional quanta, limited by the moderate coupling between the ion and the cavity, are consistent with a simple model [Phys. Rev. A 64, 033405 (2001)] without any free parameters, validating the rate equation model for cavity cooling.
Optical Sideband Cooling of Ions in a Penning Trap
NASA Astrophysics Data System (ADS)
Thompson, R. C.; Goodwin, J. F.; Stutter, G.; Segal, D. M.
Optical sideband cooling is a well-established technique for preparing trapped ions in the ground state of one or more of their motional degrees of freedom. Up to now, this technique has mainly been applied in various types of radiofrequency trap. We show in this paper that the technique is also very effective in a Penning trap, and demonstrate that our trap has an exceptionally low heating rate, due to the large size of the Penning trap electrodes and the absence of large-amplitude radiofrequency fields in the trap.
Chaotic Electron Motion Caused by Sidebands in Free Electron Lasers
1988-10-27
sideband. The total vector potential is then, A (z,t) = (1) •w (e~ )ri(krZ-Wr t) l(ksZ-Wst)] -c’-[(ex-iey)AweZ% _+V-(ex+iey)Are ikrzwr _) (ex+iey)Ase... light c, ignoring the small correction of order w 2/W 2 from the dielectric contribution of the beam. Electrostatic contributions to the fields are...mass to me and the vector potentials according to ai=IeIAi/mec2 the dimensionless Hamiltonian describing the electron motion in the fields of Eq. (1
Power-recycled Michelson interferometer with resonant sideband extraction.
Shaddock, Daniel A; Gray, Malcolm B; Mow-Lowry, Conor; McClelland, David E
2003-03-01
We present a system for the control and signal extraction of a power-recycled Michelson interferometer with resonant sideband extraction. This control system is capable of locking four degrees of freedom to a fixed point while locking the signal cavity to an arbitrary detuned point. One of the strengths of this system is that it can quickly change the instrument's frequency response without disrupting continuous operation. We report on an experimental implementation of this control system on a benchtop prototype and present broadband measurements of the prototype's frequency response for a range of signal cavity detunings.
Resolved Atomic Interaction Sidebands in an Optical Clock Transition
Bishof, M.; Lin, Y.; Swallows, M. D.; Ye, J.; Rey, A. M.; Gorshkov, A. V.
2011-06-24
We report the observation of resolved atomic interaction sidebands (ISB) in the {sup 87}Sr optical clock transition when atoms at microkelvin temperatures are confined in a two-dimensional optical lattice. The ISB are a manifestation of the strong interactions that occur between atoms confined in a quasi-one-dimensional geometry and disappear when the confinement is relaxed along one dimension. The emergence of ISB is linked to the recently observed suppression of collisional frequency shifts. At the current temperatures, the ISB can be resolved but are broad. At lower temperatures, ISB are predicted to be substantially narrower and useful spectroscopic tools in strongly interacting alkaline-earth gases.
Optical Generation and Detection of Local Nonequilibrium Phonons in Suspended Graphene
NASA Astrophysics Data System (ADS)
Sullivan, Sean; Vallabhaneni, Ajit; Kholmanov, Iskandar; Ruan, Xiulin; Murthy, Jayathi; Shi, Li
2017-03-01
The measured frequencies and intensities of different first- and second- order Raman peaks of suspended graphene are used to show that optical phonons and different acoustic phonon polarizations are driven out of local equilibrium inside a sub-micron laser spot. The experimental results are correlated with a first principles-based multiple temperature model to suggest a considerably lower equivalent local temperature of the flexural phonons than those of other phonon polarizations. The finding reveals weak coupling between the flexural modes with hot electrons and optical phonons. Since the ultrahigh intrinsic thermal conductivity of graphene has been largely attributed to contributions from the flexural phonons, the observed local non-equilibrium phenomena have important implications for understanding energy dissipation processes in graphene-based electronic and optoelectronic devices, as well as in Raman measurements of thermal transport in graphene and other two-dimensional materials.
NASA Astrophysics Data System (ADS)
Akhoondali, Hossein; Goharrizi, Arash Yazdanpanah; Sharifi, Mohammad Javad
2014-11-01
The effect of optical and acoustic phonon-scattering in the presence of line-edge-roughness (LER) on the electronic properties of ultra-scaled armchair graphene nano-ribbons (AGNRs) is investigated. Non-equilibrium Green's function formalism (NEGF) is employed using a Hamiltonian formed from tight bonding model with consideration of first and third nearest neighbors. The combined effect of phonons and line edge roughness on the transmission, transport gap, and conductance are studied for different roughness strengths and AGNR lengths. Results show edge roughness slightly reduces the onset of optical phonon emission, acoustic phonons reduce off-state conductance and optical phonons reduce on-state conductance. In both cases, the degree and behavior of reduction is totally dependent on the intensity of edge roughness. Also, in the longer AGNRs with high edge roughness intensity, phonons increase the transport gap.
Hussein, Mahmoud I.; El-Kady, Ihab; Li, Baowen; ...
2014-12-31
“Phononics” is an interdisciplinary branch of physics and engineering that deals with the behavior of phonons, and more broadly elastic and acoustic waves in similar context, and their manipulation in solids and/or fluids to benefit technological applications. Compared to resembling disciplines, such as electronics and photonics, phononics is a youthful field. It is growing at a remarkable rate, especially when viewed liberally with no limiting constraints on any particular length scale, discipline or application.
Phonon waveguides for electromechanical circuits.
Hatanaka, D; Mahboob, I; Onomitsu, K; Yamaguchi, H
2014-07-01
Nanoelectromechanical systems (NEMS), utilizing localized mechanical vibrations, have found application in sensors, signal processors and in the study of macroscopic quantum mechanics. The integration of multiple mechanical elements via electrical or optical means remains a challenge in the realization of NEMS circuits. Here, we develop a phonon waveguide using a one-dimensional array of suspended membranes that offers purely mechanical means to integrate isolated NEMS resonators. We demonstrate that the phonon waveguide can support and guide mechanical vibrations and that the periodic membrane arrangement also creates a phonon bandgap that enables control of the phonon propagation velocity. Furthermore, embedding a phonon cavity into the phonon waveguide allows mobile mechanical vibrations to be dynamically switched or transferred from the waveguide to the cavity, thereby illustrating the viability of waveguide-resonator coupling. These highly functional traits of the phonon waveguide architecture exhibit all the components necessary to permit the realization of all-phononic NEMS circuits.
Surface Phonons and Polaritons.
1976-01-01
for an impurity in the surface of a crystal could be observed in the one phonon cross section for the resonant absorption or e.ission of ,—rays by...localized at the surface. The w5 — dependence has a simple physical origin. It is well known that the cross section for scattering of bulk phonons by a...propagate. In Section II of the present Chapter we present the theory underlying the surface induced vibrational properties of crystals which we have
NASA Astrophysics Data System (ADS)
Feng, Danqi; Sun, Junqiang; Xie, Heng
2015-10-01
We propose and experimentally demonstrate a novel approach to realize tunable optical carrier-to-sideband ratio (OCSR) by introducing two radiofrequency (RF) signals with phase difference to drive a Mach-Zehnder modulator. Stimulated Brillouin scattering is adopted to remove the undesirable sideband, converting double sideband (DSB) to single sideband (SSB). By altering RF signal phase difference, wide ranges of OCSR from -23 to 44 dB and -21 to 44 dB are obtained for the DSB and SSB modulation, respectively. The operation frequency bandwidth covers from 5 to 42.3 GHz. The optimum OCSR to maximize the output RF power is also presented for the best transmission behavior. The proposed approach will be vital for optimizing the transmission performance by improving modulation efficiency and receiver sensitivity.
NASA Astrophysics Data System (ADS)
Chen, Zhao-Jiang
2015-01-01
A new kind of one-dimensional multilayer phononic heterostructure is constructed to obtain a broad acoustic omnidirectional reflection (ODR) band. The heterostructure is formed by combining finite periodic phononic crystals (PnCs) and Fibonacci (or Thue—Morse) quasiperiodic PnCs. From the numerical results performed by the transfer matrix method, it is found that the ODR bands can be enlarged obviously by using the combination of periodic and quasi-periodic PnCs. Moreover, an application of particle swarm optimization in designing and optimizing acoustic ODR bands is reported. With regards to different thickness ratios and periodic numbers in the heterostructure, we give some optimization examples and finally achieve phononic heterostructure with a very broad ODR bandwidth. The result provides a new approach to achieve broad acoustic ODR bandwidth, and will be applied in design of omnidirectional acoustic mirrors.
Cavity-type hypersonic phononic crystals
NASA Astrophysics Data System (ADS)
Sato, A.; Pennec, Y.; Yanagishita, T.; Masuda, H.; Knoll, W.; Djafari-Rouhani, B.; Fytas, G.
2012-11-01
We report on the engineering of the phonon dispersion diagram in monodomain anodic porous alumina (APA) films through the porosity and physical state of the material residing in the nanopores. Lattice symmetry and inclusion materials are theoretically identified to be the main factors which control the hypersonic acoustic wave propagation. This involves the interaction between the longitudinal and the transverse modes in the effective medium and a flat band characteristic of the material residing in the cavities. Air and filled nanopores, therefore, display markedly different dispersion relations and the inclusion materials lead to a locally resonant structural behavior uniquely determining their properties under confinement. APA films emerge as a new platform to investigate the rich acoustic phenomena of structured composite matter.
Electron–phonon coupling in hybrid lead halide perovskites
Wright, Adam D.; Verdi, Carla; Milot, Rebecca L.; Eperon, Giles E.; Pérez-Osorio, Miguel A.; Snaith, Henry J.; Giustino, Feliciano; Johnston, Michael B.; Herz, Laura M.
2016-01-01
Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH2)2PbI3, HC(NH2)2PbBr3, CH3NH3PbI3 and CH3NH3PbBr3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron–phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ∼40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites. PMID:27225329
Electron-phonon coupling in hybrid lead halide perovskites
NASA Astrophysics Data System (ADS)
Wright, Adam D.; Verdi, Carla; Milot, Rebecca L.; Eperon, Giles E.; Pérez-Osorio, Miguel A.; Snaith, Henry J.; Giustino, Feliciano; Johnston, Michael B.; Herz, Laura M.
2016-05-01
Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH2)2PbI3, HC(NH2)2PbBr3, CH3NH3PbI3 and CH3NH3PbBr3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron-phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ~40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites.
Electron-phonon coupling in hybrid lead halide perovskites.
Wright, Adam D; Verdi, Carla; Milot, Rebecca L; Eperon, Giles E; Pérez-Osorio, Miguel A; Snaith, Henry J; Giustino, Feliciano; Johnston, Michael B; Herz, Laura M
2016-05-26
Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH2)2PbI3, HC(NH2)2PbBr3, CH3NH3PbI3 and CH3NH3PbBr3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron-phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ∼40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites.
Electron-phonon interactions and the intrinsic electrical resistivity of graphene.
Park, Cheol-Hwan; Bonini, Nicola; Sohier, Thibault; Samsonidze, Georgy; Kozinsky, Boris; Calandra, Matteo; Mauri, Francesco; Marzari, Nicola
2014-03-12
We present a first-principles study of the temperature- and density-dependent intrinsic electrical resistivity of graphene. We use density-functional theory and density-functional perturbation theory together with very accurate Wannier interpolations to compute all electronic and vibrational properties and electron-phonon coupling matrix elements; the phonon-limited resistivity is then calculated within a Boltzmann-transport approach. An effective tight-binding model, validated against first-principles results, is also used to study the role of electron-electron interactions at the level of many-body perturbation theory. The results found are in excellent agreement with recent experimental data on graphene samples at high carrier densities and elucidate the role of the different phonon modes in limiting electron mobility. Moreover, we find that the resistivity arising from scattering with transverse acoustic phonons is 2.5 times higher than that from longitudinal acoustic phonons. Last, high-energy, optical, and zone-boundary phonons contribute as much as acoustic phonons to the intrinsic electrical resistivity even at room temperature and become dominant at higher temperatures.
Phonon-lifetimes in demixing systems
NASA Astrophysics Data System (ADS)
Davaasambuu, J.; Güthoff, F.; Petri, M.; Hradil, K.; Schober, H.; Ollivier, J.; Eckold, G.
2012-06-01
The dynamics of silver-alkali halide mixed single crystals (AgxNa1-xBr, x = 0.23, 0.35, 0.40 and 0.70) were studied by inelastic neutron scattering during the process of spinodal decomposition. Using the thermal three-axes spectrometer PUMA as well as the time-of-flight spectrometer IN5, the time evolution of phonons was observed in time-resolved, stroboscopic measurements. Complementary to the study of long wavelength acoustic phonons, as studied previously, we extended these investigations to Brillouin-zone boundary modes that are particularly sensitive to variations of the local structure. Starting from the homogeneous mixed phase the behaviour of these modes during demixing is observed in real-time. A simple dynamical model based on local structure variants helps to interpret the results. It is shown that the phonon lifetimes vary strongly during the phase separation and increase drastically during the coarsening process. Up to a critical size of precipitates of about 10 nm, zone-boundary modes are found to be strongly damped, while beyond the line widths are reduced to the experimental resolution. This finding leads to the conclusion that the typical mean free path of these modes is of the order of 10 nm, which corresponds to 20 unit cells.
Zarkevich, Nikolai
2014-11-24
ThermoPhonon is a stand-alone code, which can be integrated into other software packages. Typically, it is used together with a density functional theory (DFT) code (such as VASP, Wien2k, AbInit, SIESTA) and a phonon code (such as Phonopy or Phon). The workflow is the following. Molecular dynamics (MD) in a supercell at a given temperature T is performed using another code. After sufficient equilibration, the output in the form of atomic positions and forces for a large number of selected MD steps is recorded into a file. If needed, one can modify this file by applying additional constraints, such as enforced crystal symmetry or subtracted motion of the center of mass. ThermoPhonon reads the file with atomic positions and forces and writes a new file with the force constants. Force constants can be used by another code (such as Phonopy or Phon) to produce phonon spectrum for plotting, in the assumption of known equilibrium atomic positions provided in a separate file.
ERIC Educational Resources Information Center
Reid, John S.
1977-01-01
Discussed are how the thermal vibrations of a solid are described in terms of lattice waves, how these waves interact with other waves, or with themselves, and how one is led from such a description in terms of waves to the concept of a phonon. (Author/MA)
Phonon transport properties of two-dimensional group-IV materials from ab initio calculations
NASA Astrophysics Data System (ADS)
Peng, Bo; Zhang, Hao; Shao, Hezhu; Xu, Yuanfeng; Ni, Gang; Zhang, Rongjun; Zhu, Heyuan
2016-12-01
It has been argued that stanene has lowest lattice thermal conductivity among two-dimensional (2D) group-IV materials because of its largest atomic mass, weakest interatomic bonding, and enhanced ZA phonon scattering due to the breaking of an out-of-plane symmetry selection rule. However, we show that, although the lattice thermal conductivity κ for graphene, silicene, and germanene decreases monotonically with decreasing Debye temperature, unexpected higher κ is observed in stanene. By enforcing all the invariance conditions in 2D materials and including Ge 3 d and Sn 4 d electrons as valence electrons for germanene and stanene, respectively, the lattice dynamics in these materials are accurately described. A large acoustic-optical gap and the bunching of the acoustic-phonon branches significantly reduce phonon scattering in stanene, leading to higher thermal conductivity than germanene. The vibrational origin of the acoustic-optical gap can be attributed to the buckled structure. Interestingly, a buckled system has two competing influences on phonon transport: the breaking of the symmetry selection rule leads to reduced thermal conductivity, and the enlarging of the acoustic-optical gap results in enhanced thermal conductivity. The size dependence of thermal conductivity is investigated as well. In nanoribbons, the κ of silicene, germanene, and stanene is much less sensitive to size effect due to their short intrinsic phonon mean-free paths. This work sheds light on the nature of phonon transport in buckled 2D materials.
Lan, Tian; Li, Chen W.; Hellman, O.; ...
2015-08-11
Although the rutile structure of TiO2 is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly predicting a structural collapse at temperatures well below 1000 K. In this paper, inelastic neutron scattering was used to measure the temperature dependence of the phonon density of states (DOS) of rutile TiO2 from 300 to 1373 K. Surprisingly, these anomalous acoustic phonons were found to increase in frequency with temperature. First-principles calculations showed that with lattice expansion, the potentials for the anomalous acoustic phonons transform from quadratic to quartic, stabilizingmore » the rutile phase at high temperatures. In these modes, the vibrational displacements of adjacent Ti and O atoms cause variations in hybridization of 3d electrons of Ti and 2p electrons of O atoms. Finally, with thermal expansion, the energy variation in this “phonon-tracked hybridization” flattens the bottom of the interatomic potential well between Ti and O atoms, and induces a quarticity in the phonon potential.« less
Phonon properties of americium phosphide
NASA Astrophysics Data System (ADS)
Arya, B. S.; Aynyas, Mahendra; Sanyal, S. P.
2016-05-01
Phonon properties of AmP have been studied by using breathing shell models (BSM) which includes breathing motion of electrons of the Am atoms due to f-d hybridization. The phonon dispersion curves, specific heat calculated from present model. The calculated phonon dispersion curves of AmP are presented follow the same trend as observed in uranium phosphide. We discuss the significance of this approach in predicting the phonon dispersion curves of these compounds and examine the role of electron-phonon interaction.
Investigation of Sideband Index Response to Prototype Gear Tooth Damage
NASA Technical Reports Server (NTRS)
Dempsey, Paula J.
2013-01-01
The objective of this analysis was to evaluate the ability of gear condition indicators (CI) to detect contact fatigue damage on spiral bevel gear teeth. Tests were performed in the NASA Glenn Spiral Bevel Gear Fatigue Rig on eight prototype gear sets (pinion/gear). Damage was initiated and progressed on the gear and pinion teeth. Vibration data was measured during damage progression at varying torque values while varying damage modes to the gear teeth were observed and documented with inspection photos. Sideband indexes (SI) and root mean square (RMS) CIs were calculated from the time synchronous averaged vibration data. Results found that both CIs respond differently to varying torque levels, damage levels and damage modes
Sideband Rabi spectroscopy of finite-temperature trapped Bose gases
NASA Astrophysics Data System (ADS)
Allard, Baptiste; Fadel, Matteo; Schmied, Roman; Treutlein, Philipp
2016-04-01
We use Rabi spectroscopy to explore the low-energy excitation spectrum of a finite-temperature Bose gas of rubidium atoms across the phase transition to a Bose-Einstein condensate (BEC). To record this spectrum, we coherently drive the atomic population between two spin states. A small relative displacement of the spin-specific trapping potentials enables sideband transitions between different motional states. The intrinsic nonlinearity of the motional spectrum, mainly originating from two-body interactions, makes it possible to resolve and address individual excitation lines. Together with sensitive atom counting, this constitutes a feasible technique to count single excited atoms of a BEC and to determine the temperature of nearly pure condensates. As an example, we show that for a nearly pure BEC of N =800 atoms the first excited state has a population of less than five atoms, corresponding to an upper bound on the temperature of 30 nK .
All optical labeling scheme with vestigial sideband payload.
Chen, Hongwei; Chen, Minghua; Dai, Yitang; Xie, Shizhong; Zhou, Bingkun
2005-04-04
A novel scheme based on 40Gb/s vestigial sideband modulation for optical payload and label multiplex and separation in all optical label switching (AOLS) networks is firstly proposed and experimentally demonstrated. The payload is combined and separated with wavelength labels by optical filters. The experiment results show that after label separation, the power penalties of payload and label are both very little. The influence of the wavelength difference between label and payload is also discussed. The power penalty of payload can be less than 1dB as long as the wavelength difference is larger than 0.1nm. This scheme highly reduces the channel bandwidth of payload and label and is proposing to be used in future optical Internet.
Coulomb and electron-phonon interactions in metals
NASA Astrophysics Data System (ADS)
Tupitsyn, Igor S.; Mishchenko, Andrey S.; Nagaosa, Naoto; Prokof'ev, Nikolay
2016-10-01
An accurate and consistent theory of phonons in metals requires that all long-range Coulomb interactions between charged particles (electrons and ions) be treated on equal footing. So far, all attempts to deal with this nonperturbative system were relying on uncontrolled approximations in the absence of small parameters. In this paper, we develop the diagrammatic Monte Carlo approach for a two-component Coulomb system that obtains the solution to this fundamental problem in an approximation-free way by computing vertex corrections from higher-order skeleton graphs. The feasibility of the method is demonstrated by calculating the spectrum of longitudinal acoustic phonons in a simple cubic lattice, determining their sound velocity, and obtaining the phonon spectral densities by analytic continuation of the Matsubara-Green's functions. Final results are checked against the lowest-order fully self-consistent G W approximation in both adiabatic and nonadiabatic regimes.
A GaAs phononic crystal with shallow noncylindrical holes.
Petrus, Joseph A; Mathew, Reuble; Stotz, James A H
2014-02-01
A square lattice of shallow, noncylindrical holes in GaAs is shown to act as a phononic crystal (PnC) reflector. The holes are produced by wet-etching a GaAs substrate using a citric acid:H2O2 etching procedure and a photolithographed array pattern. Although nonuniform and asymmetric etch rates limit the depth and shape of the phononic crystal holes, the matrix acts as a PnC, as demonstrated by insertion loss measurements together with interferometric imaging of surface acoustic waves propagating on the GaAs surface. The measured vertical displacement induced by surface phonons compares favorably with finite-difference time-domain simulations of a PnC with rounded-square holes.
Phononic crystal plate with hollow pillars connected by thin bars
NASA Astrophysics Data System (ADS)
Jin, Yabin; Pennec, Yan; Pan, Yongdong; Djafari-Rouhani, Bahram
2017-01-01
A new type of phononic crystal plate consisting of hollow pillars on a bar-connected plate is proposed. With respect to usual pillar based phononic crystal plates, the Bragg band gap can be tuned to be much wider and extended to a sub-wavelength region, and the low frequency gap can be moved to an extremely low frequency range. Such a structure can generate quadrapolar, hexapolar and octopolar whispering-gallery modes (WGMs) inside the band gaps with very high confinement and quality factors. By filling the hollow pillars with a liquid, these WGMs, together with additional localized compressional and solid-liquid coupling modes, can be tuned either by varying the inner radius of the pillars or controlling the height of the liquid. We discuss some possible functionalities of these phononic crystals for the purpose of sensing the acoustic properties of liquids, multiplexer and wireless communication.
Dispersive Phonon Imaging in Iii-V Semiconductors.
NASA Astrophysics Data System (ADS)
Hebboul, Saad Eddine
Low-temperature transport properties of high-frequency acoustic phonons are investigated in GaAs, InSb, InP and InAs using the phonon-imaging technique. In this method, a focused laser beam provides a movable heat source on one side of a cooled crystal (<=q2 K). A single small phonon detector on the opposite face records the transmitted heat flux as a function of propagation direction. Ballistic phonons channel along directions in the crystal which are completely determined by the detailed shape of constant-energy surfaces in wavevector space. The resulting focusing patterns are characterized by sharp phonon caustics which are clearly identified from the continuous background due to scattered phonons. In the dispersive regime, where phonon wavelength is comparable to atomic spacing, the angular positions of these caustic lines are very sensitive to phonon frequency, thus providing a novel test for lattice dynamics theories. Experiments are performed with superconducting tunnel junctions and Al bolometers to probe both the high-frequency and low -frequency regimes, respectively. We find that large-k ballistic phonons give rise to distinct focusing patterns in all four types of crystals, with thicknesses varying between 0.4 and 0.8 mm. Due to isotope scattering in the bulk, tunnel-junction experiments yield well-defined caustic patterns with a dominant frequency given by the detector gap 2Delta. In InSb, where zone boundary frequencies are small (nu_ {TA} ~ 1.2 THz), the frequency dependence of the dispersive phonon focusing patterns are measured using PbTl (0.43, 0.59 THz) and PbBi (0.69, 0.73, 0.78, 0.82 THz) tunnel junction detectors. The results are interpreted with Monte Carlo calculations based on rigid, dipole, shell, and bond-charge models. Although each model yields satisfactory fits to the previously measured dispersion curves, the predicted patterns show remarkable differences in the caustic structures. This result underscores the utility of phonon imaging
Edge waves and resonances in two-dimensional phononic crystal plates
NASA Astrophysics Data System (ADS)
Hsu, Jin-Chen; Hsu, Chih-Hsun
2015-05-01
We present a numerical study on phononic band gaps and resonances occurring at the edge of a semi-infinite two-dimensional (2D) phononic crystal plate. The edge supports localized edge waves coupling to evanescent phononic plate modes that decay exponentially into the semi-infinite phononic crystal plate. The band-gap range and the number of edge-wave eigenmodes can be tailored by tuning the distance between the edge and the semi-infinite 2D phononic lattice. As a result, a phononic band gap for simultaneous edge waves and plate waves is created, and phononic cavities beside the edge can be built to support high-frequency edge resonances. We design an L3 edge cavity and analyze its resonance characteristics. Based on the band gap, high quality factor and strong confinement of resonant edge modes are achieved. The results enable enhanced control over acoustic energy flow in phononic crystal plates, which can be used in designing micro and nanoscale resonant devices and coupling of edge resonances to other types of phononic or photonic crystal cavities.
Note: Efficient generation of optical sidebands at GHz with a high-power tapered amplifier
Zappala, J. C.; Lu, Z.-T.; Bailey, K.; O’Connor, T. P.; Jiang, W.
2014-04-15
Two methods using a laser-diode tapered amplifier to produce high-power, high-efficiency optical frequency sidebands over a wide tunable frequency range are studied and compared. For a total output of 500 mW at 811 nm, 20% of the power can be placed in each of the first-order sidebands. Functionality and characterization are presented within the sideband frequency region of 0.8–2.3 GHz, and it is shown that both methods can be applied beyond this frequency range. These methods provide a versatile and effective tool for atomic physics experiments.
Gallium nitride electro-acoustic devices and acoustic metamaterials
NASA Astrophysics Data System (ADS)
Rais-Zadeh, Mina
2016-05-01
Gallium nitride (GaN) being one of a few piezoelectric semiconductors with low acoustic loss is a perfect material for electro-acoustic applications. Interactions of electrons and phonons are facilitated by the piezoelectric effect in addition to the deformation coupling in GaN, a property that can be used to implement a variety of very interesting devices and metamaterials, such as resonant transistors, acoustic amplifiers, circulators, and couplers. This talk covers theoretical basis of such devices and overviews recent advances in this technology.
Femtosecond electron imaging of defect-modulated phonon dynamics
Cremons, Daniel R.; Plemmons, Dayne A.; Flannigan, David J.
2016-01-01
Precise manipulation and control of coherent lattice oscillations via nanostructuring and phonon-wave interference has the potential to significantly impact a broad array of technologies and research areas. Resolving the dynamics of individual phonons in defect-laden materials presents an enormous challenge, however, owing to the interdependent nanoscale and ultrafast spatiotemporal scales. Here we report direct, real-space imaging of the emergence and evolution of acoustic phonons at individual defects in crystalline WSe2 and Ge. Via bright-field imaging with an ultrafast electron microscope, we are able to image the sub-picosecond nucleation and the launch of wavefronts at step edges and resolve dispersion behaviours during propagation and scattering. We discover that the appearance of speed-of-sound (for example, 6 nm ps−1) wavefronts are influenced by spatially varying nanoscale strain fields, taking on the appearance of static bend contours during propagation. These observations provide unprecedented insight into the roles played by individual atomic and nanoscale features on acoustic-phonon dynamics. PMID:27079790
Electron-phonon coupling and thermal transport in thermoelectric compound Mo3Sb7-xTex
NASA Astrophysics Data System (ADS)
Bansal, Dipanshu; Li, Chen; Said, Ayman; Abernathy, Douglas; Yan, Jiaqiang; Delaire, Olivier
Complex interactions between solid-state excitations, such as phonon-phonon, phonon-electron, and phonon-magnon couplings are often responsible for unusual material properties. In this presentation, we report on our investigations of phonon propagation and thermal transport in thermoelectric Mo3Sb7-xTex. We have performed extensive inelastic neutron and x-ray scattering measurements of phonons in Mo3Sb7-xTex, mapping the phonon dispersions and density of states, as function of temperature and composition. Our first-principles density functional theory simulations, coupled with experimental measurements, reveal the importance of electron-phonon coupling, which dominates the scattering rates over alloy disorder scattering. Doping with Te shifts the Fermi surface near the top of the valence band, suppressing screening and causing phonons to stiffen markedly. Our measurements of acoustic dispersions and linewidths, coupled with DFT simulations and models of phonon scattering enable us to quantify the impact of the electron-phonon coupling on the thermal conductivity.
Temperature induced phonon behaviour in germanium selenide thin films probed by Raman spectroscopy
NASA Astrophysics Data System (ADS)
Taube, A.; Łapińska, A.; Judek, J.; Wochtman, N.; Zdrojek, M.
2016-08-01
Here we report a detailed study of temperature-dependent phonon properties of exfoliated germanium selenide thin films (several tens of nanometers thick) probed by Raman spectroscopy in the 70-350 K temperature range. The temperature-dependent behavior of the positions and widths of the Raman modes was nonlinear. We concluded that the observed effects arise from anharmonic phonon-phonon interactions and are explained by the phenomenon of optical phonon decay into acoustic phonons. At temperatures above 200 K, the position of the Raman modes tended to be linearly dependent, and the first order temperature coefficients χ were -0.0277, -0.0197 and -0.031 cm-1 K-1 for B 3g , A g(1) and A g(2) modes, respectively.
Dispersion and absorption in one-dimensional nonlinear lattices: A resonance phonon approach
NASA Astrophysics Data System (ADS)
Xu, Lubo; Wang, Lei
2016-09-01
Based on the linear response theory, we propose a resonance phonon (r-ph) approach to study the renormalized phonons in a few one-dimensional nonlinear lattices. Compared with the existing anharmonic phonon (a-ph) approach, the dispersion relations derived from this approach agree with the expectations of the effective phonon (e-ph) theory much better. The application is also largely extended, i.e., it is applicable in many extreme situations, e.g., high frequency, high temperature, etc., where the existing one can hardly work. Furthermore, two separated phonon branches (one acoustic and one optical) with a clear gap in between can be observed by the r-ph approach in a diatomic anharmonic lattice. While only one combined branch can be detected in the same lattice with both the a-ph approach and the e-ph theory.
Inelastic x-ray scattering measurements of phonon dynamics in URu_{2}Si_{2}
Gardner, D. R.; Bonnoit, C. J.; Chisnell, R.; Said, A. H.; Leu, B. M.; Williams, Travis J.; Luke, G. M.; Lee, Y. S.
2016-02-11
In this paper, we study high-resolution inelastic x-ray scattering measurements of the acoustic phonons of URu_{2}Si_{2}. At all temperatures, the longitudinal acoustic phonon linewidths are anomalously broad at small wave vectors revealing a previously unknown anharmonicity. The phonon modes do not change significantly upon cooling into the hidden order phase. In addition, our data suggest that the increase in thermal conductivity in the hidden order phase cannot be driven by a change in phonon dispersions or lifetimes. Hence, the phonon contribution to the thermal conductivity is likely much less significant compared to that of the magnetic excitations in the low temperature phase.
Yoctocalorimetry: phonon counting in nanostructures
NASA Astrophysics Data System (ADS)
Roukes, M. L.
1999-03-01
It appears feasible with nanostructures to perform calorimetry at the level of individual thermal phonons. Here I outline an approach employing monocrystalline mesoscopic insulators, which can now be patterned from semiconductor heterostructures into complex geometries with full, three-dimensional relief. Successive application of these techniques also enables definition of integrated nanoscale thermal transducers; coupling these to a dc SQUID readout yields the requisite energy sensitivity and temporal resolution with minimal back action. The prospect of phonon counting opens intriguing experimental possibilities with analogies in quantum optics. These include fluctuation-based phonon spectroscopy, phonon shot noise in the energy relaxation of nanoscale systems, and quantum statistical phenomena such as phonon bunching and anticorrelated electron-phonon exchange.
Phonon Spectrum Engineering in Rolled-up Micro- and Nano-Architectures
Fomin, Vladimir M.; Balandin, Alexander A.
2015-10-10
We report on a possibility of efficient engineering of the acoustic phonon energy spectrum in multishell tubular structures produced by a novel high-tech method of self-organization of micro- and nano-architectures. The strain-driven roll-up procedure paved the way for novel classes of metamaterials such as single semiconductor radial micro- and nano-crystals and multi-layer spiral micro- and nano-superlattices. The acoustic phonon dispersion is determined by solving the equations of elastodynamics for InAs and GaAs material systems. It is shown that the number of shells is an important control parameter of the phonon dispersion together with the structure dimensions and acoustic impedance mismatch between the superlattice layers. The obtained results suggest that rolled up nano-architectures are promising for thermoelectric applications owing to a possibility of significant reduction of the thermal conductivity without degradation of the electronic transport.
Phonon Spectrum Engineering in Rolled-up Micro- and Nano-Architectures
Fomin, Vladimir M.; Balandin, Alexander A.
2015-10-10
We report on a possibility of efficient engineering of the acoustic phonon energy spectrum in multishell tubular structures produced by a novel high-tech method of self-organization of micro- and nano-architectures. The strain-driven roll-up procedure paved the way for novel classes of metamaterials such as single semiconductor radial micro- and nano-crystals and multi-layer spiral micro- and nano-superlattices. The acoustic phonon dispersion is determined by solving the equations of elastodynamics for InAs and GaAs material systems. It is shown that the number of shells is an important control parameter of the phonon dispersion together with the structure dimensions and acoustic impedance mismatchmore » between the superlattice layers. The obtained results suggest that rolled up nano-architectures are promising for thermoelectric applications owing to a possibility of significant reduction of the thermal conductivity without degradation of the electronic transport.« less
Vestibular schwannoma; Tumor - acoustic; Cerebellopontine angle tumor; Angle tumor; Hearing loss - acoustic; Tinnitus - acoustic ... Acoustic neuromas have been linked with the genetic disorder neurofibromatosis type 2 (NF2). Acoustic neuromas are uncommon.
Geometric tuning of thermal conductivity in three-dimensional anisotropic phononic crystals.
Wei, Zhiyong; Wehmeyer, Geoff; Dames, Chris; Chen, Yunfei
2016-10-07
Molecular dynamics simulations are performed to investigate the thermal transport properties of a three-dimensional (3D) anisotropic phononic crystal consisting of silicon nanowires and films. The calculation shows that the in-plane thermal conductivity is negatively correlated with the out-of-plane thermal conductivity upon making geometric changes, whether varying the nanowire diameter or the film thickness. This enables the anisotropy ratio of thermal conductivity to be tailored over a wide range, in some cases by more than a factor of 20. Similar trends in thermal conductivity are also observed from an independent phonon ray tracing simulation considering only diffuse boundary scattering effects, though the range of anisotropy ratios is smaller than that obtained in MD simulation. By analyzing the phonon dispersion relation with varied geometric parameters, it is found that increasing the nanowire diameter increases the out-of-plane acoustic phonon group velocities, but reduces the in-plane longitudinal and fast transverse acoustic phonon group velocities. The calculated phonon irradiation further verified the negative correlation between the in-plane and the out-of-plane thermal conductivity. The proposed 3D phononic crystal may find potential application in thermoelectrics, energy storage, catalysis and sensing applications owing to its widely tailorable thermal conductivity.
Kirschner, Matthew S.; Lethiec, Clotilde M.; Lin, Xiao-Min; Schatz, George C.; Chen, Lin X.; Schaller, Richard D.
2016-05-18
Localized surface plasmon resonances (LSPRs) arising from metallic nanoparticles offer an array of prospective applications that range from chemical sensing to biotherapies. Bipyramidal particles exhibit particularly narrow ensemble LSPR resonances that reflect small dispersity of size and shape but until recently were only synthetically accessible over a limited range of sizes with corresponding aspect ratios. Narrow size dispersion offers the opportunity to examine ensemble dynamical phenomena such as coherent phonons that induce periodic oscillations of the LSPR energy. Here, we characterize transient optical behavior of a large range of gold bipyramid sizes, as well as higher aspect ratio nanojavelin ensembles with specific attention to the lowest-order acoustic phonon mode of these nanoparticles. We report coherent phonon-driven oscillations of the LSPR position for particles with resonances spanning 670 to 1330 nm. Nanojavelins were shown to behave similarly to bipyramids but offer the prospect of separate control over LSPR energy and coherent phonon oscillation period. We develop a new methodology for quantitatively measuring mechanical expansion caused by photogenerated coherent phonons. Using this method, we find an elongation of approximately 1% per photon absorbed per unit cell and that particle expansion along the lowest frequency acoustic phonon mode is linearly proportional to excitation fluence for the fluence range studied. These characterizations provide insight regarding means to manipulate phonon period and transient mechanical deformation.
Development of a signal-extraction scheme for resonant sideband extraction
NASA Astrophysics Data System (ADS)
Kokeyama, K.; Somiya, K.; Kawazoe, F.; Sato, S.; Kawamura, S.; Sugamoto, A.
2008-12-01
As a future plan, an advanced gravitational-wave detector will employ an optical configuration of resonant sideband extraction (RSE), achieved with an additional mirror at the signal-detection port of the power-recycled Fabry Perot Michelson interferometer. To control the complex coupled cavity system, one of the most important design issues is how to extract the longitudinal control signals of the cavities. We have developed a new signal-extraction scheme which provides an appropriate sensing matrix. The new method uses two sets of sidebands: one of the sideband components satisfies the critical coupling condition for the RSE interferometer and reaches the signal-extraction port, and the other sideband is completely reflected by the Michelson interferometer. They provide a diagonalized sensing matrix and enable the RSE control to be robust.
NASA Astrophysics Data System (ADS)
Wang, Peng; Liu, Jun; Li, Fangjia; Shen, Xiong; Li, Ruxin
2015-05-01
Tunable intense multicolored femtosecond sidebands are generated in a 0.1 mm-thick sapphire plate based on cascaded four-wave mixing (CFWM) by using a spectrally broadened pulse from filamentation in air and a 806 nm fundamental pulse from a Ti:sapphire laser amplifier. By using the filamentation to extend the spectrum of one incident pulse, the experimental setup is compact and inexpensive. Furthermore, the spectra of the sidebands can be conveniently tuned by varying the input power for the filamentation generation, and even the second-order frequency upconversion sideband can maintain its output power higher than 0.2 mW during the process of tuning. The generated sidebands are observed with a spectral range from 500 to 950 nm, and each spectrum has a full width half maximum (FWHM) bandwidth above 37 nm, which have potential applications in ultrafast spectroscopy and microscopy.
Estreicher, S. K. Gibbons, T. M.; Kang, By.; Bebek, M. B.
2014-01-07
Defects in semiconductors introduce vibrational modes that are distinct from bulk modes because they are spatially localized in the vicinity of the defect. Light impurities produce high-frequency modes often visible by Fourier-transform infrared absorption or Raman spectroscopy. Their vibrational lifetimes vary by orders of magnitude and sometimes exhibit unexpectedly large isotope effects. Heavy impurities introduce low-frequency modes sometimes visible as phonon replicas in photoluminescence bands. But other defects such as surfaces or interfaces exhibit spatially localized modes (SLMs) as well. All of them can trap phonons, which ultimately decay into lower-frequency bulk phonons. When heat flows through a material containing defects, phonon trapping at localized modes followed by their decay into bulk phonons is usually described in terms of phonon scattering: defects are assumed to be static scattering centers and the properties of the defect-related SLMs modes are ignored. These dynamic properties of defects are important. In this paper, we quantify the concepts of vibrational localization and phonon trapping, distinguish between normal and anomalous decay of localized excitations, discuss the meaning of phonon scattering in real space at the atomic level, and illustrate the importance of phonon trapping in the case of heat flow at Si/Ge and Si/C interfaces.
Switchable topological phonon channels
NASA Astrophysics Data System (ADS)
Süsstrunk, Roman; Zimmermann, Philipp; Huber, Sebastian D.
2017-01-01
Guiding energy deliberately is one of the central elements in engineering and information processing. It is often achieved by designing specific transport channels in a suitable material. Topological metamaterials offer a way to construct stable and efficient channels of unprecedented versatility. However, due to their stability it can be tricky to terminate them or to temporarily shut them off without changing the material properties massively. While a lot of effort was put into realizing mechanical topological metamaterials, almost no works deal with manipulating their edge channels in sight of applications. Here, we take a step in this direction, by taking advantage of local symmetry breaking potentials to build a switchable topological phonon channel.
Imaging carrier and phonon transport in Si using ultrashort optical pulses
David H. Hurley; O. B. Wright; O. Matsuda; B. E. McCandless; S. Shinde
2009-01-01
A series of experiments have been conducted that microscopically image thermal diffusion and surface acoustic phonon propagation within a single crystallite of a polycrystalline Si sample. The experimental approach employs ultrashort optical pulses to generate an electron-hole plasma and a second probe pulse is used to image the evolution of the plasma. By decomposing the signal into a component that varies with delay time and a steady state component that varies with pump modulation frequency, the respective influence of carrier recombination and thermal diffusion are identified. Additionally, the coherent surface acoustic phonon component to the signal is imaged using a Sagnac interferometer to monitor optical phase.
Dynamic Rabi sidebands in laser-generated microplasmas: Tunability and control
Compton, R.; Filin, A.; Levis, R. J.; Romanov, D. A.
2011-05-15
Broadband, coherent radiation in the optical-frequency range is generated using microplasma channels in atmospheric gases in a pump-probe experiment. A microplasma medium is created in a gas by a focused intense femtosecond pump pulse. A picosecond probe pulse then interacts with this microplasma channel, producing broad, coherent sidebands that are associated with luminescence lines and are redshifted and blueshifted with respect to the laser carrier frequency. These sidebands originate from the induced Rabi oscillations between pairs of excited states that are coupled by the probe pulse. Thus the sideband radiation intensity tracks the microplasma evolution. The sidebands arise from broad and tunable Rabi shifts corresponding to varying values of the electric-field magnitude in the probe pulse. The {approx}10{sup 10} W cm{sup -2} probe beam creates a maximum sideband shift of >90 meV from the carrier frequency, resulting in an effective bandwidth of 200 meV. The sidebands can be tuned and controlled by the intensity and temporal profile of the probe pulse. The fact that the coherence is observed in a microplasma demonstrates that Rabi cycling is possible at high temperature with moderately high laser intensities as long as transitions close to the driving frequency ({Delta}{approx}2%{omega}{sub c}) are available. Plasma excitation combined with Rabi-shifting measurements also serves as a means to simultaneously extract quantitative ratios for the transition-dipole moments between multiple sets of highly excited states with transitions in the optical regime.
Lee, Dong-Joon; Whitaker, John F
2008-09-15
We demonstrate that harmonic sidebands of an electro-optic modulator's driving frequency can be used as the local oscillator in a photonic down-mixing process in order to significantly enhance the bandwidth of near-field, electro-optic, microwave measurements. The creation of second- and third-order-harmonic modulation sidebands on a laser-diode output are described, with heterodyne down-conversion of microwave signals taking place within an electro-optic sensor crystal. The measurement bandwidth of an electro-optic microwave probe can thus be enhanced by as much as a factor of three with respect to the use of conventional, fundamental-harmonic sidebands. Carrier-sideband analysis from the measured optical spectrum indicates that millimeter-wave-frequency local-oscillator sidebands can be created using a Ku-band electro-optic modulator and that the electro-optic-signal-modulation depth can be enhanced by suppressing the light-beam carrier component. Transverse near-field distributions from high frequency patch antennas are extracted using both second- and third-order-harmonic sidebands.
Giant nonlinearity via breaking parity-time symmetry: A route to low-threshold phonon diodes
NASA Astrophysics Data System (ADS)
Zhang, Jing; Peng, Bo; Ã-zdemir, Şahin Kaya; Liu, Yu-xi; Jing, Hui; Lü, Xin-you; Liu, Yu-long; Yang, Lan; Nori, Franco
2015-09-01
Nonreciprocal devices that permit wave transmission in only one direction are indispensible in many fields of science including, e.g., electronics, optics, acoustics, and thermodynamics. Manipulating phonons using such nonreciprocal devices may have a range of applications such as phonon diodes, transistors, switches, etc. One way of achieving nonreciprocal phononic devices is to use materials with strong nonlinear response to phonons. However, it is not easy to obtain the required strong mechanical nonlinearity, especially for few-phonon situations. Here we present a general mechanism to amplify nonlinearity using parity-time (PT )-symmetric structures, and show that an on-chip microscale phonon diode can be fabricated using a PT -symmetric mechanical system, in which a lossy mechanical resonator with very weak mechanical nonlinearity is coupled to a mechanical resonator with mechanical gain but no mechanical nonlinearity. When this coupled system transits from the PT -symmetric regime to the broken-PT -symmetric regime, the mechanical nonlinearity is transferred from the lossy resonator to the one with gain, and the effective nonlinearity of the system is significantly enhanced. This enhanced mechanical nonlinearity is almost lossless because of the gain-loss balance induced by the PT -symmetric structure. Such an enhanced lossless mechanical nonlinearity is then used to control the direction of phonon propagation, and can greatly decrease (by over three orders of magnitude) the threshold of the input-field intensity necessary to observe the unidirectional phonon transport. We propose an experimentally realizable lossless low-threshold phonon diode of this type. Our study opens up perspectives for constructing on-chip few-phonon devices and hybrid phonon-photon components.
Basic phononic diagnostic measurements in fluid columns
NASA Astrophysics Data System (ADS)
Hazony, D.; Hazony, Y.
2010-07-01
A pre-selected 21 MHz ultrasonic transducer was used to produce characteristic pulses, arbitrarily similar to the quantum-mechanical concept of a phonon, describable as having a single-frequency modulated Gaussian shape. The propagation of such pulses in water-acoustic channels was studied in conjunction with nonlinear regression analysis and an Erlangian model for size distribution of molecular aggregates. Experimental results obtained distinguish between surface and bulk phenomena and provide quantitative measures of an average molecular cluster size in water. The relevance of the Erlangian model, in studying the near front of the channel, provides a significant distinction between the behavior of pure water and Ringer's solution of water. The inherent consistency between the various results re-enforces the theoretical approach, implying new venues for future research.
Optimal design of tunable phononic bandgap plates under equibiaxial stretch
NASA Astrophysics Data System (ADS)
Hedayatrasa, Saeid; Abhary, Kazem; Uddin, M. S.; Guest, James K.
2016-05-01
Design and application of phononic crystal (PhCr) acoustic metamaterials has been a topic with tremendous growth of interest in the last decade due to their promising capabilities to manipulate acoustic and elastodynamic waves. Phononic controllability of waves through a particular PhCr is limited only to the spectrums located within its fixed bandgap frequency. Hence the ability to tune a PhCr is desired to add functionality over its variable bandgap frequency or for switchability. Deformation induced bandgap tunability of elastomeric PhCr solids and plates with prescribed topology have been studied by other researchers. Principally the internal stress state and distorted geometry of a deformed phononic crystal plate (PhP) changes its effective stiffness and leads to deformation induced tunability of resultant modal band structure. Thus the microstructural topology of a PhP can be altered so that specific tunability features are met through prescribed deformation. In the present study novel tunable PhPs of this kind with optimized bandgap efficiency-tunability of guided waves are computationally explored and evaluated. Low loss transmission of guided waves throughout thin walled structures makes them ideal for fabrication of low loss ultrasound devices and structural health monitoring purposes. Various tunability targets are defined to enhance or degrade complete bandgaps of plate waves through macroscopic tensile deformation. Elastomeric hyperelastic material is considered which enables recoverable micromechanical deformation under tuning finite stretch. Phononic tunability through stable deformation of phononic lattice is specifically required and so any topology showing buckling instability under assumed deformation is disregarded. Nondominated sorting genetic algorithm (GA) NSGA-II is adopted for evolutionary multiobjective topology optimization of hypothesized tunable PhP with square symmetric unit-cell and relevant topologies are analyzed through finite
Phonon analog of topological nodal semimetals
NASA Astrophysics Data System (ADS)
Po, Hoi Chun; Bahri, Yasaman; Vishwanath, Ashvin
2016-05-01
Topological band structures in electronic systems like topological insulators and semimetals give rise to highly unusual physical properties. Analogous topological effects have also been discussed in bosonic systems, but the novel phenomena typically occur only when the system is excited by finite-frequency probes. A mapping recently proposed by C. L. Kane and T. C. Lubensky [Nat. Phys. 10, 39 (2014), 10.1038/nphys2835], however, establishes a closer correspondence. It relates the zero-frequency excitations of mechanical systems to topological zero modes of fermions that appear at the edges of an otherwise gapped system. Here we generalize the mapping to systems with an intrinsically gapless bulk. In particular, we construct mechanical counterparts of topological semimetals. The resulting gapless bulk modes are physically distinct from the usual acoustic Goldstone phonons and appear even in the absence of continuous translation invariance. Moreover, the zero-frequency phonon modes feature adjustable momenta and are topologically protected as long as the lattice coordination is unchanged. Such protected soft modes with tunable wave vector may be useful in designing mechanical structures with fault-tolerant properties.
Thermoelectric amplification of phonons in graphene
NASA Astrophysics Data System (ADS)
Dompreh, K. A.; Mensah, N. G.; Mensah, S. Y.; Fosuhene, S. K.
2016-06-01
Amplification of acoustic in-plane phonons due to an external temperature gradient (∇T) in single-layer graphene (SLG) was studied theoretically. The threshold temperature gradient (∇ T ) 0 g and the threshold voltage (V T ) 0 g in SLG were evaluated. For T = 77 K , the calculated value for (∇ T ) 0 g = 746.8 K / cm and (V T ) 0 g = 6.6 mV . The calculation was done in the hypersound regime. Further, the dependence of the normalized amplification ( Γ / Γ 0 ) on the frequency ω q and ∇ T / T were evaluated numerically and presented graphically. The calculated threshold temperature gradient (V T ) 0 g for SLG was higher than that obtained for homogeneous semiconductors (n-InSb) (∇ T ) 0 hom ≈ 10 3 K / cm , superlattices (∇ T ) 0 S L ≈ 384 K / cm , and cylindrical quantum wire (∇ T ) 0 c q w ≈ 10 2 K / cm . This makes SLG a much better material for thermoelectric phonon amplification.
An Artificial Ising System with Phononic Excitations
NASA Astrophysics Data System (ADS)
Ghaffari, Hamed; Griffith, W. Ashley; Benson, Philip; Nasseri, M. H. B.; Young, R. Paul
Many intractable systems and problems can be reduced to a system of interacting spins. Here, we report mapping collective phononic excitations from different sources of crystal vibrations to spin systems. The phononic excitations in our experiments are due to micro and nano cracking (yielding crackling noises due to lattice distortion). We develop real time mapping of the multi-array senores to a network-space and then mapping the excitation- networks to spin-like systems. We show that new mapped system satisfies the quench (impulsive) characteristics of the Ising model in 2D classical spin systems. In particular, we show that our artificial Ising system transits between two ground states and approaching the critical point accompanies with a very short time frozen regime, inducing formation of domains separated by kinks. For a cubic-test under a true triaxial test (3D case), we map the system to a 6-spin ring under a transversal-driving field where using functional multiplex networks, the vector components of the spin are inferred (i.e., XY model). By visualization of spin patterns of the ring per each event, we demonstrate that ``kinks'' (as defects) proliferate when system approach from above to its critical point. We support our observations with employing recorded acoustic excitations during distortion of crystal lattices in nano-indentation tests on different crystals (silicon and graphite), triaxial loading test on rock (poly-crystal) samples and a true 3D triaxial test.
Raman electron spin-lattice relaxation with the Debye-type and with real phonon spectra in crystals
NASA Astrophysics Data System (ADS)
Hoffmann, Stanislaw K.; Lijewski, Stefan
2013-02-01
Electron spin-lattice relaxation temperature dependence was measured for Ti2+ (S = 1) and for Cu2+ (S = 1/2) ions in SrF2 single crystal by electron spin echo method in temperature range 4-109 K. The spin relaxation was governed by the two-phonon Raman processes. The relaxation theory is outlined and presented in a form suitable for applying with real phonon spectra. The experimental relaxation results were described using Debye-type phonon spectrum and the real phonon spectrum of SrF2 crystal. The Debye approximation does not fit well the results for SrF2 both at low and at high temperature. The relaxation rate is faster than that predicted by Debye-type phonon spectrum at low temperatures where excess of lattice vibrations over the Debye model exists but is slower at higher temperatures (above 50 K) where density of phonon states continuously decreases when approaching to the maximal acoustic phonon frequency. The expected deviation from Debye approximation was analyzed also for Cu2+ in NaCl and MgSiO3 crystals for which phonon spectra are available. The fitting with the real phonon spectrum allowed us to calculate spin-phonon coupling parameter as 267 cm-1 for Ti2+ and 1285 cm-1 for Cu2+ in SrF2.
ERIC Educational Resources Information Center
Hamilton, M. W.
2007-01-01
A nonlinear aspect of the acousto-optic interaction that is analogous to multi-photon absorption is discussed. An experiment is described in which the second-order acousto-optically scattered intensity is measured and found to scale with the square of the acoustic intensity. This experiment using a commercially available acousto-optic modulator is…
Structural engineering of three-dimensional phononic crystals
NASA Astrophysics Data System (ADS)
Delpero, Tommaso; Schoenwald, Stefan; Zemp, Armin; Bergamini, Andrea
2016-02-01
Artificially-structured materials are attracting the research interest of a growing community of scientists for the possibility to develop novel materials with advantageous properties that arise from the ability to tailor the propagation of elastic waves, and thus energy, through them. In this work, we propose a three-dimensional phononic crystal whose unit cell has been engineered to obtain a strong wave-attenuation band in the middle of the acoustic frequency range. The combination of its acoustic properties with the dimensions of the unit cell and its static mechanical properties makes it an interesting material for possibly several applications in civil and mechanical engineering, for instance as the core of an acoustically insulating sandwich panel. A sample of this crystal has been manufactured and experimentally tested with respect to its acoustic transmissibility. The performance of the phononic crystal core is remarkable both in terms of amplitude reduction in the transmissibility and width of the attenuation band. A parametric study has been finally conducted on selected geometrical parameters of the unit cell and on their effect on the macroscopic properties of the crystal. This work represents an application-oriented example of how the macroscopic properties of an artificially-structured material can be designed, according to specific needs, by a conventional engineering of its unit cell.
Topological phononic states of underwater sound based on coupled ring resonators
He, Cheng; Li, Zheng; Ni, Xu; Sun, Xiao-Chen; Yu, Si-Yuan; Lu, Ming-Hui Liu, Xiao-Ping; Chen, Yan-Feng
2016-01-18
We report a design of topological phononic states for underwater sound using arrays of acoustic coupled ring resonators. In each individual ring resonator, two degenerate acoustic modes, corresponding to clockwise and counter-clockwise propagation, are treated as opposite pseudospins. The gapless edge states arise in the bandgap resulting in protected pseudospin-dependent sound transportation, which is a phononic analogue of the quantum spin Hall effect. We also investigate the robustness of the topological sound state, suggesting that the observed pseudospin-dependent sound transportation remains unless the introduced defects facilitate coupling between the clockwise and counter-clockwise modes (in other words, the original mode degeneracy is broken). The topological engineering of sound transportation will certainly promise unique design for next generation of acoustic devices in sound guiding and switching, especially for underwater acoustic devices.
Multi-band asymmetric acoustic transmission in a bended waveguide with multiple mechanisms
NASA Astrophysics Data System (ADS)
Huang, Yu-lei; Sun, Hong-xiang; Xia, Jian-ping; Yuan, Shou-qi; Ding, Xin-lei
2016-07-01
We report the realization of a multi-band device of the asymmetric acoustic transmission by placing a phononic crystal inside a bended waveguide immersed in water, as determined both experimentally and numerically. The asymmetric acoustic transmission exists in three frequency bands below 500 kHz induced by multiple mechanisms. Besides the band gap of the phononic crystal, we also introduce the deaf mode and interaction between the phononic crystal and waveguide. More importantly, this asymmetric transmission can be systematically controlled by mechanically rotating the square rods of the phononic crystal. The device has the advantages of multiple band, broader bandwidth, and adjustable property, showing promising applications in ultrasonic devices.
NASA Astrophysics Data System (ADS)
Wong, Joe
2004-03-01
The phonon spectra of plutonium and its alloys have been sought after in the past few decades following the discovery of this actinide element in 1941, but with no success. This was due to a combination of the high neutron absorption cross section of 239Pu, the common isotope, and non-availability of large single crystals of any Pu-bearing materials. We have recent designed a high resolution inelastic x-ray scattering experiment using a bright synchrotron x-ray beam at the European Sychrotron Radiation Facility (ESRF), Grenoble and mapped the full phonon dispersion curves of an fcc delta-phase polycrystalline Pu-Ga alloy (1). Several unusual features including, a large elastic anisotropy, a small shear elastic modulus C', a Kohn-like anomaly in the T1[011] branch, and a pronounced softening of the [111] transverse modes are found. These features can be related to the phase transitions of plutonium and to strong coupling between the lattice structure and the 5f valence instabilities. Our results also provide a critical test for theoretical treatments of highly correlated 5f electron systems as exemplified by recent dynamical mean field theory (DMFT) calculations for d-plutonium.(2) This work was performed in collaboration with Dr. M. Krisch (ESRF)) and Prof. T.-C. Chiang (UIU), and under the auspices of the U. S. Department of Energy by the University of California, Lawrence Livermore National Laboratory under Contract No. W-7405-Eng-48. 1. Joe Wong et al. Science, vol.301, 1078 (2003) 2. X. Dai et al. Science, vol.300, 953 (2003)
Dynamics of a vertical cavity quantum cascade phonon laser structure
NASA Astrophysics Data System (ADS)
Maryam, W.; Akimov, A. V.; Campion, R. P.; Kent, A. J.
2013-07-01
Driven primarily by scientific curiosity, but also by the potential applications of intense sources of coherent sound, researchers have targeted the phonon laser (saser) since the invention of the optical laser over 50 years ago. Here we fabricate a vertical cavity structure designed to operate as a saser oscillator device at a frequency of 325 GHz. It is based on a semiconductor superlattice gain medium, inside a multimode cavity between two acoustic Bragg reflectors. We measure the acoustic output of the device as a function of time after applying electrical pumping. The emission builds in intensity reaching a steady state on a timescale of order 0.1 μs. We show that the results are consistent with a model of the dynamics of a saser cavity exactly analogous to the models used for describing laser dynamics. We also obtain estimates for the gain coefficient, steady-state acoustic power output and efficiency of the device.
THz Acoustic Spectroscopy by using Double Quantum Wells and Ultrafast Optical Spectroscopy
Wei, Fan Jun; Yeh, Yu-Hsiang; Sheu, Jinn-Kong; Lin, Kung-Hsuan
2016-01-01
GaN is a pivotal material for acoustic transducers and acoustic spectroscopy in the THz regime, but its THz phonon properties have not been experimentally and comprehensively studied. In this report, we demonstrate how to use double quantum wells as a THz acoustic transducer for measuring generated acoustic phonons and deriving a broadband acoustic spectrum with continuous frequencies. We experimentally investigated the sub-THz frequency dependence of acoustic attenuation (i.e., phonon mean-free paths) in GaN, in addition to its physical origins such as anharmonic scattering, defect scattering, and boundary scattering. A new upper limit of attenuation caused by anharmonic scattering, which is lower than previously reported values, was obtained. Our results should be noteworthy for THz acoustic spectroscopy and for gaining a fundamental understanding of heat conduction. PMID:27346494
Confinement of phonon propagation in laser deposited tungsten/polycarbonate multilayers
NASA Astrophysics Data System (ADS)
Döring, Florian; Ulrichs, Henning; Pagel, Sinja; Müller, Markus; Mansurova, Maria; Müller, Matthias; Eberl, Christian; Erichsen, Torben; Huebner, Dennis; Vana, Philipp; Mann, Klaus; Münzenberg, Markus; Krebs, Hans-Ulrich
2016-09-01
Nanoscale multilayer thin films of W and PC (Polycarbonate) show, due to the great difference of the components’ characteristics, fascinating properties for a variety of possible applications and provide an interesting research field, but are hard to fabricate with low layer thicknesses. Because of the great acoustic mismatch between the two materials, such nanoscale structures are promising candidates for new phononic materials, where phonon propagation is strongly reduced. In this article we show for the first time that W/PC-multilayers can indeed be grown with high quality by pulsed laser deposition. We analyzed the polymer properties depending on the laser fluence used for deposition, which enabled us to find best experimental conditions for the fabrication of high-acoustic-mismatch W/PC multilayers. The multilayers were analyzed by fs pump-probe spectroscopy showing that phonon dynamics on the ps time-scale can strongly be tailored by structural design. While already periodic multilayers exhibit strong phonon localization, especially aperiodic structures present outstandingly low phonon propagation properties making such 1D-layered W/PC nano-structures interesting for new phononic applications.
Phonon spectra of alkali metals
NASA Astrophysics Data System (ADS)
Zeković, S.; Vukajlović, F.; Veljković, V.
1982-10-01
In this work we used a simple local model pseudopotential which includes screening for the phonon spectra calculations of alkali metals. The results obtained are in very good agreement with experimental data. In some branches of phonon spectra the differences between theoretical and experimental results are within 1-2%, while the maximum error is about 6%. The suggested form of the pseudopotential allows us to describe the phonon spectra of Na, K and Rb with only one, and, at the same time, a unique, parameter. In this case, the maximum disagreements from experiment are 9% for Na, 8% for K and 7% for Rb.
Electron-Phonon Coupling and Energy Flow in a Simple Metal beyond the Two-Temperature Approximation
NASA Astrophysics Data System (ADS)
Waldecker, Lutz; Bertoni, Roman; Ernstorfer, Ralph; Vorberger, Jan
2016-04-01
The electron-phonon coupling and the corresponding energy exchange are investigated experimentally and by ab initio theory in nonequilibrium states of the free-electron metal aluminium. The temporal evolution of the atomic mean-squared displacement in laser-excited thin freestanding films is monitored by femtosecond electron diffraction. The electron-phonon coupling strength is obtained for a range of electronic and lattice temperatures from density functional theory molecular dynamics simulations. The electron-phonon coupling parameter extracted from the experimental data in the framework of a two-temperature model (TTM) deviates significantly from the ab initio values. We introduce a nonthermal lattice model (NLM) for describing nonthermal phonon distributions as a sum of thermal distributions of the three phonon branches. The contributions of individual phonon branches to the electron-phonon coupling are considered independently and found to be dominated by longitudinal acoustic phonons. Using all material parameters from first-principles calculations except the phonon-phonon coupling strength, the prediction of the energy transfer from electrons to phonons by the NLM is in excellent agreement with time-resolved diffraction data. Our results suggest that the TTM is insufficient for describing the microscopic energy flow even for simple metals like aluminium and that the determination of the electron-phonon coupling constant from time-resolved experiments by means of the TTM leads to incorrect values. In contrast, the NLM describing transient phonon populations by three parameters appears to be a sufficient model for quantitatively describing electron-lattice equilibration in aluminium. We discuss the general applicability of the NLM and provide a criterion for the suitability of the two-temperature approximation for other metals.
Ultra-pure digital sideband separation at sub-millimeter wavelengths
NASA Astrophysics Data System (ADS)
Finger, R.; Mena, F. P.; Baryshev, A.; Khudchenko, A.; Rodriguez, R.; Huaracan, E.; Alvear, A.; Barkhof, J.; Hesper, R.; Bronfman, L.
2015-12-01
Context. Deep spectral-line surveys in the mm and sub-mm range can detect thousands of lines per band uncovering the rich chemistry of molecular clouds, star forming regions and circumstellar envelopes, among others objects. The ability to study the faintest features of spectroscopic observation is, nevertheless, limited by a number of factors. The most important are the source complexity (line density), limited spectral resolution and insufficient sideband (image) rejection (SRR). Dual sideband (2SB) millimeter receivers separate upper and lower sideband rejecting the unwanted image by about 15 dB, but they are difficult to build and, until now, only feasible up to about 500 GHz (equivalent to ALMA Band 8). For example ALMA Bands 9 (602-720 GHz) and 10 (787-950 GHz) are currently double sideband (DSB) receivers. Aims: This article reports the implementation of an ALMA Band 9 2SB prototype receiver that makes use of a new technique called calibrated digital sideband separation. The new method promises to ease the manufacturing of 2SB receivers, dramatically increase sideband rejection and allow 2SB instruments at the high frequencies currently covered only by DSB or bolometric detectors. Methods: We made use of a Field Programmable Gate Array (FPGA) and fast analog-to-digital converters (ADCs) to measure and calibrate the receiver's front end phase and amplitude imbalances to achieve sideband separation beyond the possibilities of purely analog receivers. The technique could in principle allow the operation of 2SB receivers even when only imbalanced front ends can be built, particularly at very high frequencies. Results: This digital 2SB receiver shows an average sideband rejection of 45.9 dB while small portions of the band drop below 40 dB. The performance is 27 dB (a factor of 500) better than the average performance of the proof-of-concept Band 9 purely-analog 2SB prototype receiver developed by SRON. Conclusions: We demonstrate that this technique has the
Murakami, Miwa; Arai, Hajime; Uchimoto, Yoshiharu; Ogumi, Zempachi
2013-06-01
We examine applicability of rotation-synchronized Delays Alternating with Nutation for Tailored Excitation (rs-DANTE) to a crowded sideband spectrum spreading over a few 100 kHz by the paramagnetic interaction. It is shown that rs-DANTE can be used to excite (6)Li spinning sideband manifolds of the three crystallographic Li sites (2b, 4h, and 2c) in a magic-angle spinning (MAS) spectrum of (6)Li-enriched Li2MnO3. The observed lineshape is insensitive to rf inhomogeneiety, thus indicating practical applicability of rs-DANTE to a paramagnetic system. Each sideband pattern can be described by the paramagnetic anisotropies evaluated by taking the electron-(6)Li dipolar interactions into account. The isotropic chemical shift for each site can thus be obtained by comparing the experimental sideband pattern to the calculated one. It is therefore possible by this approach to obtain both isotropic and anisotropic shift information. Further effects of structural disorder in Li2MnO3 on the isotropic shift and the sideband pattern are discussed.
NASA Astrophysics Data System (ADS)
Murakami, Miwa; Arai, Hajime; Uchimoto, Yoshiharu; Ogumi, Zempachi
2013-06-01
We examine applicability of rotation-synchronized Delays Alternating with Nutation for Tailored Excitation (rs-DANTE) to a crowded sideband spectrum spreading over a few 100 kHz by the paramagnetic interaction. It is shown that rs-DANTE can be used to excite 6Li spinning sideband manifolds of the three crystallographic Li sites (2b, 4h, and 2c) in a magic-angle spinning (MAS) spectrum of 6Li-enriched Li2MnO3. The observed lineshape is insensitive to rf inhomogeneiety, thus indicating practical applicability of rs-DANTE to a paramagnetic system. Each sideband pattern can be described by the paramagnetic anisotropies evaluated by taking the electron-6Li dipolar interactions into account. The isotropic chemical shift for each site can thus be obtained by comparing the experimental sideband pattern to the calculated one. It is therefore possible by this approach to obtain both isotropic and anisotropic shift information. Further effects of structural disorder in Li2MnO3 on the isotropic shift and the sideband pattern are discussed.
Experimental study of the influence of wind on Benjamin-Feir sideband instability
NASA Technical Reports Server (NTRS)
Bliven, L. F.; Huang, N. E.; Long, S. R.
1986-01-01
A laboratory investigation of the influence of wind on the evolution of mechanically generated regular (m.g.r.) waves is reported. Surface elevation measurements were made at four fetches for steep (0.1 less than ak(bar) less than 0.2, 2 Hz) m.g.r. waves, moderate (15 less than u(asterisk) less than 25 cm/s, 3-6 Hz) wind waves, and combinations of the m.g.r. and wind waves. The m.g.r. wave spectra exhibit Benjamin-Feir sidebands that grow exponentially with fetch and whose growth rate increases as the initial wave steepness increases. As fetch increases for the wind cases, total energy increases and the frequency of the spectral maximum downshifts, but no spectral lines representing Benjamin-Feir sidebands were detected even though the wave steepness and fetch were similar to the m.g.r. waves whose spectra displayed sidebands. As wind speed increased over the m.g.r. waves, sideband magnitude, sideband growth rate, and low-frequency perturbation components associated with the instability mechanism were reduced.
A theoretical and experimental investigation of modulation sidebands of planetary gear sets
NASA Astrophysics Data System (ADS)
Inalpolat, M.; Kahraman, A.
2009-06-01
In this paper, a simplified mathematical model is proposed to describe the mechanisms leading to modulation sidebands of planetary gear sets. The model includes key system parameters such as number of planets, planet position angles, and planet phasing relationships defined by the position angles and the number of teeth of the gears. The model is used to simulate a wide range of gear sets to show that they can be classified in five distinct groups based on their sideband behavior in terms of their frequencies and amplitudes. A special experimental planetary gear set-up is developed and planetary gear sets from of three of these five groups are procured. A methodology is developed to demonstrate modulation sidebands from the ring (internal) gear radial acceleration measurements. For each case, sets of ring gear acceleration measurements at various speed and torque conditions are presented to demonstrate rich sideband activity that agrees well with the model predictions. At the end, based on results of the parametric studies and experiments, general rules on modulation sidebands of planetary gear sets are proposed.
Control of Spectral Interference Patterns in Broad Rabi Sidebands: Terahertz Quasi-Comb Structures
NASA Astrophysics Data System (ADS)
Romanov, Dmitri; Filin, Alex; Levis, Robert
2015-05-01
Coherent broadband radiation in the form of Rabi sidebands with an effective bandwidth ~ 200 meV is generated in atmospheric-pressure gases in pump-probe experiments. The dynamic Rabi sidebands show characteristic fringe patterns of spatial-spectral interference, whose variable contrast is affected by decoherence processes. The spectrum envelope, the fringe contrast, and the fringe spacing variation in these patterns can be controlled by the intensity and shape of the probe pulse. We demonstrate such control experimentally and report analytic and numerical investigation of possibilities to produce a comb-like fringe structure. The sideband envelope is mainly determined by the sharpness of the driving probe pulse. The fringe contrast, defined by the maximum-to-minimum difference, depends strongly on the asymmetry of the driving pulse. The variation of inter-peak distance within a sideband was controlled using the temporal shape of the driving pulse. In a particular case of blue-shifted sideband emitted by excited oxygen atoms driven by a picosecond pulse of 800 nm carrier wavelength and ~ 0.05 TW/ cm2 intensity, a super-Gaussian pulse shape leads to almost equidistant fringes producing a comb-like spectrum over the interval from 1.60 to 1.66 eV. This work is supported through the Air Force Office of Scientific Research, MURI grant FA9550-10-1-0561.
Wong, Joe; Krisch, M.; Farber, D.; Occelli, F.; Schwartz, A.; Chiang, T.C.; Wall, M.; Boro, C.; Xu, Ruqing
2010-11-16
Plutonium (Pu) is well known to have complex and unique physico-chemical properties. Notably, the pure metal exhibits six solid-state phase transformations with large volume expansions and contractions along the way to the liquid state: {alpha} {yields} {beta} {yields} {gamma} {yields} {delta} {yields} {delta}{prime} {yields} {var_epsilon} {yields} liquid. Unalloyed Pu melts at a relatively low temperature {approx}640 C to yield a higher density liquid than that of the solid from which it melts, (Figure 1). Detailed understanding of the properties of plutonium and plutonium-based alloys is critical for the safe handling, utilization, and long-term storage of these important, but highly toxic materials. However, both technical and and safety issues have made experimental observations extremely difficult. Phonon dispersion curves (PDCs) are key experimenta l data to the understanding of the basic properties of Pu materials such as: force constants, sound velocities, elastic constants, thermodynamics, phase stability, electron-phonon coupling, structural relaxation, etc. However, phonon dispersion curves (PDCs) in plutonium (Pu) and its alloys have defied measurement for the past few decades since the discovery of this element in 1941. This is due to a combination of the high thermal-neutron absorption cross section of plutonium and the inability to grow the large single crystals (with dimensions of a few millimeters) necessary for inelastic neutron scattering. Theoretical simulations of the Pu PDC continue to be hampered by the lack of suitable inter -atomic potentials. Thus, until recently the PDCs for Pu and its alloys have remained unknown experimentally and theoretically. The experimental limitations have recently been overcome by using a tightly focused undulator x-ray micro-beam scattered from single -grain domains in polycrystalline specimens. This experimental approach has been applied successfully to map the complete PDCs of an fcc d-Pu-Ga alloy using the
Low-energy phonons and superconductivity in Sn0.8In0.2Te
NASA Astrophysics Data System (ADS)
Xu, Zhijun; Schneeloch, J. A.; Zhong, R. D.; Rodriguez-Rivera, J. A.; Harriger, L. W.; Birgeneau, R. J.; Gu, G. D.; Tranquada, J. M.; Xu, Guangyong
2015-02-01
We present neutron scattering measurements on low-energy phonons from a superconducting (Tc=2.7 K ) Sn0.8In0.2Te single-crystal sample. The longitudinal acoustic phonon mode and one transverse acoustic branch have been mapped out around the (002) Bragg peak for temperatures of 1.7 and 4.2 K. We observe a substantial energy width of the transverse phonons at energies comparable to twice the superconducting gap; however, there is no change in this width between the superconducting and normal states, and the precise origin of this energy width anomaly is not entirely clear. We also confirm that the compound is well ordered, with no indications of structural instability.
Granato, A.V.
1987-01-01
Acoustic technique have proven to be very useful in getting basic information on the configuration and dynamics of defects. Although the technique is indirect, the sensitivity is such that it often competes very favorably with more direct techniques such as neutron, x-ray, or phonon scattering. The symmetry information that comes directly from polarization control often also proves decisive in determining configurations. Many of the concepts that have been developed in explaining the various effects that have been seen in dislocation and point defect studies have proven also to be very useful when taken over almost directly into other areas of physics. 11 refs., 7 figs.
NASA Astrophysics Data System (ADS)
Allen, Philip B.; Nery, Jean Paul
2017-01-01
At low temperature, the experimental gap of silicon decreases as Eg(T ) =Eg(0 ) -A T4 . The main reason is electron-phonon renormalization. The physics behind the T4-power law is more complex than has been realized. Renormalization at low T by intraband scattering requires a nonadiabatic treatment in order to correctly include acoustic phonons and avoid divergences from piezoacoustic phonon interactions. The result is an unexpected low T term Eg(0 ) +A'Tp with positive coefficient A', and power p =4 for nonpiezoelectric materials, and power p =2 for piezoelectric materials. The acoustic phonons in piezoelectric semiconductors generate a piezoelectric field, modifying the electron-phonon coupling. However, at higher T , thermally excited acoustic phonons of energy ℏ vsq and intraband excitation energies ɛq-ɛ0=ℏ2q2/2 m* become comparable in size. Above this temperature, the low q and higher q intraband acoustic phonon contributions to Tp rapidly cancel, leaving little thermal effect. Then the contribution from interband scattering by acoustic phonons is dominant. This has the power law T4 for both nonpiezoelectric and piezoelectric semiconductors. The shift can then have either sign, but usually reduces the size of gaps as T increases. It arises after cancellation of the T2 terms that appear separately in Debye-Waller and Fan parts of the acoustic phonon interband renormalization. The cancellation occurs because of the acoustic sum rule.
25th Anniversary Article: Ordered Polymer Structures for the Engineering of Photons and Phonons
Lee, Jae-Hwang; Koh, Cheong Yang; Singer, Jonathan P; Jeon, Seog-Jin; Maldovan, Martin; Stein, Ori; Thomas, Edwin L
2014-01-01
The engineering of optical and acoustic material functionalities via construction of ordered local and global architectures on various length scales commensurate with and well below the characteristic length scales of photons and phonons in the material is an indispensable and powerful means to develop novel materials. In the current mature status of photonics, polymers hold a pivotal role in various application areas such as light-emission, sensing, energy, and displays, with exclusive advantages despite their relatively low dielectric constants. Moreover, in the nascent field of phononics, polymers are expected to be a superior material platform due to the ability for readily fabricated complex polymer structures possessing a wide range of mechanical behaviors, complete phononic bandgaps, and resonant architectures. In this review, polymer-centric photonic and phononic crystals and metamaterials are highlighted, and basic concepts, fabrication techniques, selected functional polymers, applications, and emerging ideas are introduced. PMID:24338738
25th anniversary article: ordered polymer structures for the engineering of photons and phonons.
Lee, Jae-Hwang; Koh, Cheong Yang; Singer, Jonathan P; Jeon, Seog-Jin; Maldovan, Martin; Stein, Ori; Thomas, Edwin L
2014-01-01
The engineering of optical and acoustic material functionalities via construction of ordered local and global architectures on various length scales commensurate with and well below the characteristic length scales of photons and phonons in the material is an indispensable and powerful means to develop novel materials. In the current mature status of photonics, polymers hold a pivotal role in various application areas such as light-emission, sensing, energy, and displays, with exclusive advantages despite their relatively low dielectric constants. Moreover, in the nascent field of phononics, polymers are expected to be a superior material platform due to the ability for readily fabricated complex polymer structures possessing a wide range of mechanical behaviors, complete phononic bandgaps, and resonant architectures. In this review, polymer-centric photonic and phononic crystals and metamaterials are highlighted, and basic concepts, fabrication techniques, selected functional polymers, applications, and emerging ideas are introduced.
Phonon symmetries in hexagonal boron nitride probed by incoherent light emission
NASA Astrophysics Data System (ADS)
Vuong, T. Q. P.; Cassabois, G.; Valvin, P.; Jacques, V.; Van Der Lee, A.; Zobelli, A.; Watanabe, K.; Taniguchi, T.; Gil, B.
2017-03-01
Layered compounds are stacks of weakly bound two-dimensional atomic crystals, with a prototypal hexagonal structure in graphene, transition metal dichalcogenides and boron nitride. This crystalline anisotropy results in vibrational modes with specific symmetries depending on the in-plane or out-of-plane atomic displacements. We show that polarization-resolved photoluminescence measurements in hexagonal boron nitride reflect the phonon symmetries in this layered semiconductor. Experiments performed with a detection on the sample edge, perpendicular to the c-axis, reveal the strong polarization-dependence of the emission lines corresponding to the recombination assisted by the three acoustic phonon modes. We elucidate the dipole orientation of the fundamental indirect exciton. We demonstrate evidence of the so-far missing phonon replica due to the optical out-of-plane phonon mode.
Band structures of two dimensional solid/air hierarchical phononic crystals
NASA Astrophysics Data System (ADS)
Xu, Y. L.; Tian, X. G.; Chen, C. Q.
2012-06-01
The hierarchical phononic crystals to be considered show a two-order “hierarchical” feature, which consists of square array arranged macroscopic periodic unit cells with each unit cell itself including four sub-units. Propagation of acoustic wave in such two dimensional solid/air phononic crystals is investigated by the finite element method (FEM) with the Bloch theory. Their band structure, wave filtering property, and the physical mechanism responsible for the broadened band gap are explored. The corresponding ordinary phononic crystal without hierarchical feature is used for comparison. Obtained results show that the solid/air hierarchical phononic crystals possess tunable outstanding band gap features, which are favorable for applications such as sound insulation and vibration attenuation.
Coupling of nitrogen vacancy centres in nanodiamonds by means of phonons
NASA Astrophysics Data System (ADS)
Albrecht, A.; Retzker, A.; Jelezko, F.; Plenio, M. B.
2013-08-01
Realizing controlled quantum dynamics via the magnetic interactions between colour centres in diamond remains a challenge despite recent demonstrations for nanometre separated pairs. Here we propose to use the intrinsic acoustical phonons in diamond as a data bus for accomplishing this task. We show that for nanodiamonds the electron-phonon coupling can take significant values that together with mode frequencies in the THz range can serve as a resource for conditional gate operations. Based on these results, we analyse how to use this phonon-induced interaction for constructing quantum gates among the electron-spin triplet ground states, introducing the phonon dependence via Raman transitions. Combined with decoupling pulses this offers the possibility for creating entangled states within nanodiamonds on the scale of several tens of nanometres, a promising prerequisite for quantum sensing applications.
NASA Astrophysics Data System (ADS)
Chen, Meng; Jiang, Heng; Feng, Yafei; Wang, Yuren
2014-12-01
We experimentally and theoretically investigated the mechanisms of acoustic absorption in phononic glass to optimize its properties. First, we experimentally studied its locally resonant absorption mechanism. From these results, we attributed its strong sound attenuation to its locally resonant units and its broadband absorption to its networked structure. These experiments also indicated that the porosity and thickness of the phononic glass must be tuned to achieve the best sound absorption at given frequencies. Then, using lumped-mass methods, we studied how the absorption bandgaps of the phononic glass were affected by various factors, including the porosity and the properties of the coating materials. These calculations gave optimal ranges for selecting the porosity, modulus of the coating material, and ratio of the compliant coating to the stiff matrix to achieve absorption bandgaps in the range of 6-30 kHz. This paper provides guidelines for designing phononic glasses with proper structures and component materials to work in specific frequency ranges.
Phonon dynamics of neptunium chalcogenides
NASA Astrophysics Data System (ADS)
Aynyas, Mahendra; Rukmangad, Aditi; Arya, Balwant S.; Sanyal, Sankar P.
2012-06-01
We have performed phonon calculations of Neptunium Chalcogenides (NpX) (X= S, Se, Te) based on breathing shell model (BSM) which includes breathing motion of electron of the Np-atoms due to f-d hybridization. The model predicts that the short range breathing phenomenon play a dominant role in the phonon properties. We also report, for the first time specific heat for these compounds.
Electron and Phonon Dynamics in Hexagonal Pd Nanosheets and Ag/Pd/Ag Sandwich Nanoplates.
Wang, Li; Sagaguchi, Takuya; Okuhata, Tomoki; Tsuboi, Motohiro; Tamai, Naoto
2017-02-28
Pd and its hybrid nanostructures have attracted considerable attention over the past decade, with both catalytic and plasmonic properties. The electron and phonon properties directly govern conversion efficiencies in applications such as energy collectors and photocatalysts. We report the dynamic processes of electron-phonon coupling and coherent acoustic phonon vibration in hexagonal Pd nanosheets and Ag/Pd/Ag sandwich nanoplates using transient absorption spectroscopy. The electron-phonon coupling constant of Pd nanosheets, GPd-nanosheet (8.7 × 10(17) W/(m(3)·K)) is larger than that of the bulk GPd (5.0 × 10(17) W/(m(3)·K)). The effective coupling constant Geff of Ag/Pd/Ag nanoplates decreases with increasing Ag shell thickness, finally approaching the bulk GAg. The variation of Geff is explained in terms of reduced density of states near Fermi level of Pd nanosheets with 1.8 nm ultrathin thickness. Coherent acoustic phonon vibration in Pd nanosheets is assigned to a fundamental breathing mode, similar to the vibration of benzene. The period increases with increasing Ag shell thickness. For Ag/Pd/Ag nanoplates with 20 nm thick Ag shells, the vibrational mode is ascribed to a quasi-extensional mode. The results show that the modes of the coherent acoustic phonon vibration transform with the geometric variation of Pd nanosheets and Ag/Pd/Ag nanoplates. Our results represent an understanding of quantum-confinement related electron dynamics and bulk-like phonon kinetics in the ultrathin Pd nanosheets and their hybrid nanostructures.
Isotope scattering and phonon thermal conductivity in light atom compounds: LiH and LiF
NASA Astrophysics Data System (ADS)
Lindsay, L.
2016-11-01
Engineered isotope variation is a pathway toward modulating lattice thermal conductivity (κ) of a material through changes in phonon-isotope scattering. The effects of isotope variation on intrinsic thermal resistance is little explored, as varying isotopes have relatively small differences in mass and thus do not affect bulk phonon dispersions. However, for light elements, isotope mass variation can be relatively large (e.g., hydrogen and deuterium). Using a first principles Peierls-Boltzmann transport equation approach, the effects of isotope variance on lattice thermal transport in ultra-low-mass compound materials LiH and LiF are characterized. The isotope mass variance modifies the intrinsic thermal resistance via modulation of acoustic and optic phonon frequencies, while phonon-isotope scattering from mass disorder plays only a minor role. This leads to some unusual cases where κ values of isotopically pure systems (6LiH ,7L i2H , and 6LiF ) are lower than the values from their counterparts with naturally occurring isotopes and phonon-isotope scattering. However, these κ differences are relatively small. The effects of temperature-driven lattice expansion on phonon dispersions and calculated κ are also discussed. This paper provides insight into lattice thermal conductivity modulation with mass variation and the interplay of intrinsic phonon-phonon and phonon-isotope scattering in interesting light atom systems.
Isotope scattering and phonon thermal conductivity in light atom compounds: LiH and LiF
Lindsay, Lucas R.
2016-11-08
Engineered isotope variation is a pathway toward modulating lattice thermal conductivity (κ) of a material through changes in phonon-isotope scattering. The effects of isotope variation on intrinsic thermal resistance is little explored, as varying isotopes have relatively small differences in mass and thus do not affect bulk phonon dispersions. However, for light elements isotope mass variation can be relatively large (e.g., hydrogen and deuterium). Using a first principles Peierls-Boltzmann transport equation approach the effects of isotope variance on lattice thermal transport in ultra-low-mass compound materials LiH and LiF are characterized. The isotope mass variance modifies the intrinsic thermal resistance viamore » modulation of acoustic and optic phonon frequencies, while phonon-isotope scattering from mass disorder plays only a minor role. This leads to some unusual cases where values of isotopically pure systems (6LiH, 7Li2H and 6LiF) are lower than the values from their counterparts with naturally occurring isotopes and phonon-isotope scattering. However, these differences are relatively small. The effects of temperature-driven lattice expansion on phonon dispersions and calculated κ are also discussed. This work provides insight into lattice thermal conductivity modulation with mass variation and the interplay of intrinsic phonon-phonon and phonon-isotope scattering in interesting light atom systems.« less
Isotope scattering and phonon thermal conductivity in light atom compounds: LiH and LiF
Lindsay, Lucas R.
2016-11-08
Engineered isotope variation is a pathway toward modulating lattice thermal conductivity (κ) of a material through changes in phonon-isotope scattering. The effects of isotope variation on intrinsic thermal resistance is little explored, as varying isotopes have relatively small differences in mass and thus do not affect bulk phonon dispersions. However, for light elements isotope mass variation can be relatively large (e.g., hydrogen and deuterium). Using a first principles Peierls-Boltzmann transport equation approach the effects of isotope variance on lattice thermal transport in ultra-low-mass compound materials LiH and LiF are characterized. The isotope mass variance modifies the intrinsic thermal resistance via modulation of acoustic and optic phonon frequencies, while phonon-isotope scattering from mass disorder plays only a minor role. This leads to some unusual cases where values of isotopically pure systems (^{6}LiH, ^{7}Li^{2}H and ^{6}LiF) are lower than the values from their counterparts with naturally occurring isotopes and phonon-isotope scattering. However, these differences are relatively small. The effects of temperature-driven lattice expansion on phonon dispersions and calculated κ are also discussed. This work provides insight into lattice thermal conductivity modulation with mass variation and the interplay of intrinsic phonon-phonon and phonon-isotope scattering in interesting light atom systems.
Resolved Sideband Spectroscopy and Cooling of Strontium in a 532-nm Optical Lattice
NASA Astrophysics Data System (ADS)
Aman, James; Hill, Joshua; Killian, T. C.
2016-05-01
Resolved sideband cooling is a powerful and well established technique for driving ultracold atoms in optical lattices to the motional ground state of individual lattice sites. Here we present spectroscopy of the narrow 5s21S0 --> 5 s 5 p3P1 transition for neutral strontium-84 in a 532nm optical lattice. Resolved red- and blue-detuned sidebands are observed corresponding to changes in the motional state in the lattice sites. Driving the red sideband, we demonstrate cooling into the ground state, which increases the initial phase-space density before forced evaporative cooling. This is a promising technique for improving the production of strontium quantum degenerate gases. Research supported by the Robert A, Welch Foundation under Grant No. C-1844.
Sensitivity-enhanced FBG demodulation system with multi-sideband filtering method
NASA Astrophysics Data System (ADS)
Xiong, YanLing; Ren, NaiKui; Wu, MingZe; Liang, Huan; Han, JunSheng; Yang, WenLong
2017-01-01
A multi-sideband filtering demodulation scheme with enhanced high sensitivity was proposed to demodulate weak fiber Bragg grating signals, and a novel data processing method was employed to reduce the influence of the background noise. The relationship of the sensing sensitivity, number of sidebands, and their slope coefficients were researched theoretically, numerically, and experimentally. The results showed that the sensing sensitivity was in proportion to the number of the sidebands and their slope coefficients. The power sensitivities for single and double CWDMs demodulating FBG in the experimental system were 6.960 dB/nm and 15.187 dB/nm, respectively, which were in agreement with the theoretical results. In addition, the data processing method we used to obtain the optical power was experimentally proven to be better than the method of directly measuring the optical power because it reduces the background noise.
Efficient generation of broad Raman sidebands in an index-guided photonic crystal fiber.
Li, Ying; Hou, Jing; Jiang, Zongfu; Leng, Jinyong
2013-04-01
The efficient generation of broad Raman sidebands is experimentally demonstrated in a short piece of index-guided photonic crystal fiber, which is pumped by a high-peak-power pulse near the zero-dispersion wavelength and seeded by a continuous-wave Stokes signal centered at 1117 nm. The Raman sidebands generated via stimulated Raman scattering and cascaded four-wave mixing contain five Stokes and six anti-Stokes peaks and span from 827 to 1398 nm, and the 3 dB linewidth for each peak is smaller than 1 nm. However, the pure Raman sidebands are largely dependent on the pulse pump power as well as the fiber length.
Phonon thermal properties of graphene from molecular dynamics using different potentials
NASA Astrophysics Data System (ADS)
Zou, Ji-Hang; Ye, Zhen-Qiang; Cao, Bing-Yang
2016-10-01
Phonon thermal transport in graphene has attracted significant interest in recent years. Phonon thermal properties of graphene are investigated by molecular dynamics simulations using the Tersoff, Tersoff-2010, REBO, and AIREBO potentials. By calculating the phonon properties and thermal conductivity of graphene, the performance of the potentials is evaluated based on comparisons with experimental data. It shows that the Tersoff-2010 and REBO display better dispersion curves for graphene than the original Tersoff and AIREBO. The Tersoff-2010 correctly provides the Γ point phonon velocities of the LA and TA branches as well as the G peak frequency with a value of 46 THz. In addition, the acoustic phonon relaxation time derived from the Tersoff-2010 satisfies the ideal relation "τ-1 ∝ ν2." It is also found that the Tersoff-2010 provides the highest graphene thermal conductivity among the used potentials, and estimates about 30.0% contribution for flexural phonons to the total thermal conductivity. By comparison, the Tersoff-2010 potential is demonstrated to be the most suitable one to describe the phonon thermal properties of graphene.
Nonlinear control of high-frequency phonons in spider silk
NASA Astrophysics Data System (ADS)
Schneider, Dirk; Gomopoulos, Nikolaos; Koh, Cheong Y.; Papadopoulos, Periklis; Kremer, Friedrich; Thomas, Edwin L.; Fytas, George
2016-10-01
Spider dragline silk possesses superior mechanical properties compared with synthetic polymers with similar chemical structure due to its hierarchical structure comprised of partially crystalline oriented nanofibrils. To date, silk’s dynamic mechanical properties have been largely unexplored. Here we report an indirect hypersonic phononic bandgap and an anomalous dispersion of the acoustic-like branch from inelastic (Brillouin) light scattering experiments under varying applied elastic strains. We show the mechanical nonlinearity of the silk structure generates a unique region of negative group velocity, that together with the global (mechanical) anisotropy provides novel symmetry conditions for gap formation. The phononic bandgap and dispersion show strong nonlinear strain-dependent behaviour. Exploiting material nonlinearity along with tailored structural anisotropy could be a new design paradigm to access new types of dynamic behaviour.
Giant Anharmonic Phonon Scattering in PbTe
Delaire, Olivier A; Ma, Jie; Marty, Karol J; May, Andrew F; McGuire, Michael A; Singh, David J; Lumsden, Mark D; Sales, Brian C; Du, Mao-Hua; Ehlers, Georg; Podlesnyak, Andrey A
2011-01-01
Understanding the microscopic processes affecting the bulk thermal conductivity is crucial to develop more efficient thermoelectric materials. PbTe is currently one of the leading thermoelectric materials, largely thanks to its low thermal conductivity. However, the origin of this low thermal conductivity in a simple rocksalt structure has so far been elusive. Using a combination of inelastic neutron scattering measurements and first-principles computations of the phonons, we identify a strong anharmonic coupling between the ferroelectric transverse optic (TO) mode and the longitudinal acoustic (LA) modes in PbTe. This interaction extends over a large portion of reciprocal space, and directly affects the heat-carrying LA phonons. The LA-TO anharmonic coupling is likely to play a central role in explaining the low thermal conductivity of PbTe. The present results provide a microscopic picture of why many good thermoelectric materials are found near a lattice instability of the ferroelectric type.
Anomalous phonon characteristics of unconventional novel III-N superlattices
Talwar, Devki N.
2014-03-31
Comprehensive results of atomic vibrations are reported in the unconventional short-period zb BN/GaN superlatices (SLs) by exploiting a rigid-ion-model and taking into account both the short- and long-range Coulomb interactions. Besides anisotropic mode behavior of optical phonons, our study provided evidence of acoustic-mode anti-crossing, mini-gap formation, confinement as well as BN-like modes falling within the gap that separates optical phonon bands of the two materials. A bond-polarizability scheme is employed within the second-nearest-neighbor linear-chain model to simulate the Raman intensity profiles of BN/GaN SLs revealing major expected trends of the vibrational characteristics observed experimentally in many conventional superlattice systems while eliciting some interesting contrasts.
Sideband elimination and high efficiencies in a strongly tapered FEL amplifier
Bhattacharjee, A.; Chen, J.
1995-12-31
Recently, an analytical theory has shown that sideband instabilities can be eliminated in a strongly tapered FEL amplifier, leading to high efficiencies. It is found that a drastic suppression of the sideband spectrum occurs due to a continuous detuning effect which causes the real frequency of the most unstable sideband mode to vary continuously along the wiggler axis in the presence of a strong taper, with the consequence that no sideband can grow significantly before it is tuned away. Assuming extremely strongly pre-bunched beams with zero thermal spread, ideal efficiencies exceeding 60% were predicted by the theory with sideband intensities suppressed by nearly eight orders of magnitude with respect to the intensity of the primary signal. The theoretical predictions have been tested and verified by a one-dimensional numerical simulation. The numerical simulations permit us to go beyond the scope of the analytical model and allow us to examine (i) if optimization of strongly tapered wiggler configurations can allow us to achieve the desired high efficiencies within acceptable length constraints, and (ii) whether the high ideal efficiencies predicted by theory survive in the presence of partial pre-bunching and finite thermal spread of electron beams. By experimenting with different tapering schemes, we have found interesting strongly tapered configurations in which the accessible electron phase-space area remains nearly constant, with realistic assumptions on pre-bunching and thermal spread of the electron beam. In particular, for parameters representative of the Livermore experiments we obtain efficiencies in the rage 40-50% with thermal spreads in the range 0.5-1 % and pre-bunched electron phases in the range 2 {pi}/ 3 using a wiggler 5 meters long. The optical quality of the radiation produced is free of parasitic sideband instabilities which do not grow beyond noise levels.
Control of spectral interference patterns in broad Rabi sidebands toward quasi-comb structures.
Romanov, D A; Filin, A I; Levis, R J
2015-03-01
The pattern of spectral interference fringes in broad dynamic Rabi sidebands allows for a considerable degree of control by shaping the picosecond driving pulse. We demonstrate experimental evidence of such control and report an analytic and numerical investigation of possibilities to control the fringe pattern to produce a comb-like optical structure. The temporal phase and amplitude shaping of a picosecond driving pulse influence the spectrum envelope, fringe contrast, and fringe spacing variation in the sideband spectra. The sideband spectrum envelope depends on the sharpness of the driving pulse, that is, on the rate at which the temporal distance between the leading and trailing edges grows away from the pulse maximum. Increasing this parameter reduces the variation of the envelope amplitude across the sideband. The fringe contrast, defined by the maximum-to-minimum difference, depends strongly on the asymmetry of the driving pulse. The imbalance between the leading and trailing edges leads to a decrease of the contrast. The variation of interpeak distance within a sideband was controlled using the temporal shape of the driving pulse. In the particular case of a blue-shifted sideband emitted by excited oxygen atoms driven by a picosecond pulse of 800 nm carrier wavelength and ∼5×10¹⁰ W cm⁻² intensity, a Gaussian pulse shape results in an interpeak distance increasing almost five times over the interval from 1.60 to 1.66 eV, whereas a super-Gaussian shape leads to almost equidistant fringes producing a comb-like spectrum.
Lan, Tian; Li, Chen W.; Hellman, O.; Kim, D. S.; Muñoz, Jorge A.; Smith, Hillary; Abernathy, Douglas L.; Fultz, B.
2015-08-11
Although the rutile structure of TiO_{2} is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly predicting a structural collapse at temperatures well below 1000 K. In this paper, inelastic neutron scattering was used to measure the temperature dependence of the phonon density of states (DOS) of rutile TiO_{2} from 300 to 1373 K. Surprisingly, these anomalous acoustic phonons were found to increase in frequency with temperature. First-principles calculations showed that with lattice expansion, the potentials for the anomalous acoustic phonons transform from quadratic to quartic, stabilizing the rutile phase at high temperatures. In these modes, the vibrational displacements of adjacent Ti and O atoms cause variations in hybridization of 3d electrons of Ti and 2p electrons of O atoms. Finally, with thermal expansion, the energy variation in this “phonon-tracked hybridization” flattens the bottom of the interatomic potential well between Ti and O atoms, and induces a quarticity in the phonon potential.
Method and means for generation of tunable laser sidebands in the far-infrared region
NASA Technical Reports Server (NTRS)
Pickett, Herbert M. (Inventor); Farhoomand, Jam (Inventor)
1987-01-01
A method for generating tunable far-infrared radiation is described. The apparatus includes a Schottky-barrier diode which has one side coupled through a conductor to a waveguide that carries a tunable microwave frequency; the diode has an opposite side which is coupled through a radiating whisker to a bias source. Infrared light is directed at the diode, and infrared light with tunable sidebands is radiated by the whisker through an open space to a reflector. The original infrared is separated from a tunable infrared sideband by a polarizing Michelson interferometer.
Spinning sidebands from chemical shift anisotropy in 13C MAS imaging.
Scheler, U; Blümich, B; Spiess, H W
1993-07-01
Solid state imaging by 13C MAS imaging is described. The spinning sidebands occurring at moderate spinning speeds, which disturb the images, can be suppressed by TOSS. For rigid solids the spatial resolution that can be achieved in this way is better than that of 1H images at the same spinning speed. Spatially resolved spectra with or without spinning sidebands can likewise be recorded providing information about the isotropic and the anisotropic chemical shifts which can be exploited for the study of structure, order and dynamics. The techniques are demonstrated on a phantom made with 13C-labelled glycine.
Interference measurements on amplitude compandored single sideband (ACSB) land mobil radio
NASA Astrophysics Data System (ADS)
Wootton, H.
1983-06-01
The National Telecommunications and Information Administration (NTIA) funded the ECAC to conduct adjacent-signal interference tests on a new radio system technology that shows promise of allowing smaller channel spacing in the Government land mobile radio band (162-174 MHz). The system tested was an amplitude compandored single-sideband radio (ACSB) manufactured by Sideband Technology, Inc. This report presents the adjacent-signal interference (ASI) result which will be employed by NTIA in evaluation of the potential usage of the ACSB technology in the Government land mobile radio band.
Si3N4 Optomechanical Crystals in the Resolved-sideband Regime
2014-01-27
Si3N4 optomechanical crystals in the resolved-sideband regime M. Davanço,1,2,a) S. Ates,1,3,b) Y. Liu,1,3,c) and K. Srinivasan1 1Center for...November 2013; accepted 13 December 2013; published online 27 January 2014) We demonstrate sideband-resolved Si3N4 optomechanical crystals supporting...which leads to reduced Qo for large N. As an alternative to Si, Si3N4 is a potentially advanta- geous material for OMCs: it does not exhibit two-photon
Optical single-sideband OFDM transmission based on a two-segment EAM.
Cheng, Hsuan-Lin; Chen, Wei-Hung; Wei, Chia-Chien; Chiu, Yi-Jen
2015-01-26
This paper presents a novel optical single-sideband (SSB) OFDM modulation scheme using a two-segment electro-absorption modulator (EAM). Differences in the chirp characteristics of two segments of the EAM make it possible to design driving signals capable of suppressing one of the optical sidebands, such that the optical OFDM signal does not suffer from frequency-selective power fading following dispersive fiber transmission. Our experiment results demonstrate optical OFDM transmissions at 13.5-Gbps over a 0 ∼ 200-km IM/DD system without the need for dispersion compensation and distance-dependent bit- and power-loading.
Sideband excitation of trapped ions by rapid adiabatic passage for manipulation of motional states
Watanabe, T.; Nomura, S.; Toyoda, K.; Urabe, S.
2011-09-15
We describe an analysis and experimental results of the manipulation of motional states of a single trapped {sup 40}Ca{sup +} ion based on sideband excitation by rapid adiabatic passage. When the sideband transition is excited by rapid adiabatic passage, adiabaticity may be affected by ac Stark shifts. We investigate the influence of ac Stark shifts and compensate for these shifts with an additional laser field. This makes the population transfer by rapid adiabatic passage more robust with respect to experimental parameters. Finally, we manipulate the motional states and generate motional Fock states of a single {sup 40}Ca{sup +} ion by rapid adiabatic passage with ac Stark compensation.
A Tone-Aided/Dual Vestigial Sideband (TA/DVSB) system for mobile satellite channels
NASA Technical Reports Server (NTRS)
Saulnier, Gary J.; Millar, Gilbert M.; Depaolo, Anthony D.
1990-01-01
Tone-aided modulation is one way of combatting the effects of multipath fading and Doppler frequency shifts. A new tone-aided modulation format for M-ary phase-shift keyed signals (MPSK) is discussed. A spectral null for the placement of the tone is created in the center of the MPSK signal by translating the upper sideband upwards in frequency by the same amount. The key element of the system is the algorithm for recombining the data sidebands in the receiver, a function that is performed by a specialized phase-locked loop (PLL). The system structure is discussed and simulation results showing the PLL acquisition performance are presented.
NASA Astrophysics Data System (ADS)
Liu, Na; Chen, Xue; Ju, Cheng; Hui, Rongqing
2014-11-01
The intersymbol interference caused by dispersion, chirp, and a vestigial sideband filter in intensity modulation and a direct detection single carrier system is analyzed theoretically and numerically. An iterative nonlinear intersymbol interference cancellation technique is proposed and experimentally demonstrated in a 40-Gbps 16-QAM Mach-Zehnder modulator-based vestigial sideband intensity modulation and direct detection half-cycle Nyquist-subcarrier modulation system over a 100-km uncompensated standard single-mode fiber transmission for the first time. The experimental results show that 2.2-dB receiver sensitivity improvement is obtained at the forward error correction limit by using the iterative technique.
Comparing the anomalous phonons in Fe(Te,Se) and (Fe,Ni)(Te,Se) via neutron scattering
NASA Astrophysics Data System (ADS)
Schneeloch, John; Xu, Zhijun; Gu, Genda; Zaliznyak, Igor; Winn, Barry; Rodriguez-Rivera, Jose; Birgeneau, Robert; Xu, Guangyong; Tranquada, John
We studied the anomalous acoustic-type phonons in the Fe(Te,Se) iron-based superconductor family that arise from the (100) Bragg peak, which is forbidden according to the reported crystal structure for these materials. Inelastic neutron scattering was performed on superconducting and non-superconducting crystals of various compositions. The (100) phonons were much weaker in a non-superconducting nickel-doped crystal than in a superconducting crystal with similar selenium fraction, but comparison with another non-superconducting crystal suggests the difference is not simply related to superconductivity. This composition dependence was observed for both transverse and longitudinal phonons. The temperature dependences of the (100) phonons resembled those of conventional phonons. We will discuss these results and possible explanations for the relation between composition and lattice dynamics in this system.
Zhernenkov, Mikhail; Bolmatov, Dima; Soloviov, Dmitry; ...
2016-05-12
We report the high resolution inelastic x-ray study of the in-plane phonon excitations in dipalmitoyl phosphatidylcholine (DPPC) above and below main transition temperature. In the Lβ' gel phase, we observe high frequency longitudinal phonon mode previously predicted by the molecular dynamics simulations and for the first time, we reveal low frequency weakly dispersive transverse acoustic mode which softens and exhibits a low-frequency phonon gap when the DPPC lipid transitions into the Lα fluid phase. The phonon softening of the high frequency longitudinal excitations and the transformation of the transverse excitations upon the phase transition from the Lβ' to Lα phasemore » is explained within the framework of the phonon theory of liquids. These findings illustrate the importance of the collective dynamics of biomembranes and reveal that hydrocarbon tails can act as an efficient mediator in controlling the passive transport across the bilayer plane.« less
Anomalous Infrared Spectra of Hybridized Phonons in Type-I Clathrate Ba8Ga16Ge30
NASA Astrophysics Data System (ADS)
Iwamoto, Kei; Kushibiki, Shunsuke; Honda, Hironori; Kajitani, Shuhei; Mori, Tatsuya; Matsumoto, Hideki; Toyota, Naoki; Suekuni, Koichiro; Avila, Marcos A.; Takabatake, Toshiro
2013-02-01
The optical conductivity spectra of the rattling phonons in the clathrate Ba8Ga16Ge30 are investigated in detail by use of the terahertz time-domain spectroscopy. The experiment has revealed that the lowest-lying vibrational mode of Ba(2)2+ ions consist of a sharp Lorentzian peak at 1.2 THz superimposed on a broad tail weighted in the lower frequency regime around 1.0 THz. With decreasing temperature, an unexpected linewidth broadening of the phonon peak is observed, together with monotonic softening of the phonon peak and enhancement of the tail structure. These observed anomalies are discussed in terms of impurity scattering effects on the hybridized phonon system of rattling and acoustic phonons.
Neutron inelastic scattering measurements of low-energy phonons in the multiferroic BiFeO_{3}
Schneeloch, John A.; Xu, Zhijun; Wen, Jinsheng; Gehring, P. M.; Stock, C.; Matsuda, Masaaki; Winn, Barry L.; Gu, Genda; Shapiro, Stephen M.; Birgeneau, R. J.; Ushiyama, T.; Yanagisawa, Y.; Tomioka, Y.; Ito, T.; Xu, Guangyong
2015-02-10
In this study, we present neutron inelastic scattering measurements of the low-energy phonons in single crystal BiFeO_{3}. The dispersions of the three acoustic phonon modes (LA along [100], TA_{1} along [010], and TA_{2} along [110]) and two low-energy optic phonon modes (LO and TO_{1}) have been mapped out between 300 and 700 K. Elastic constants are extracted from the phonon measurements. The energy linewidths of both TA phonons at the zone boundary clearly broaden when the system is warmed toward the magnetic ordering temperature T_{N}=640 K. In conclusion, this suggests that the magnetic order and low-energy lattice dynamics in this multiferroic material are coupled.
Neutron inelastic scattering measurements of low-energy phonons in the multiferroic BiFeO3
Schneeloch, John A.; Xu, Zhijun; Wen, Jinsheng; ...
2015-02-10
In this study, we present neutron inelastic scattering measurements of the low-energy phonons in single crystal BiFeO3. The dispersions of the three acoustic phonon modes (LA along [100], TA1 along [010], and TA2 along [110]) and two low-energy optic phonon modes (LO and TO1) have been mapped out between 300 and 700 K. Elastic constants are extracted from the phonon measurements. The energy linewidths of both TA phonons at the zone boundary clearly broaden when the system is warmed toward the magnetic ordering temperature TN=640 K. In conclusion, this suggests that the magnetic order and low-energy lattice dynamics in thismore » multiferroic material are coupled.« less
Biswas, Tutul; Ghosh, Tarun Kanti
2013-07-03
We theoretically study the phonon-drag contribution to the thermoelectric power and the hot-electron energy-loss rate in a Rashba spin-orbit coupled two-dimensional electron system in the Bloch-Gruneisen (BG) regime. We assume that electrons interact with longitudinal acoustic phonons through a deformation potential and with both longitudinal and transverse acoustic phonons through a piezoelectric potential. The effect of the Rashba spin-orbit interaction on the magnitude and temperature dependence of the phonon-drag thermoelectric power and hot-electron energy-loss rate is discussed. We numerically extract the exponent of temperature dependence of the phonon-drag thermopower and the energy-loss rate. We find that the exponents are suppressed due to the presence of the Rashba spin-orbit coupling.
NASA Astrophysics Data System (ADS)
Feng, Tianli; Ruan, Xiulin; Ye, Zhenqiang; Cao, Bingyang
2015-06-01
The spectral phonon properties in defected graphene have been unclear due to the lack of advanced techniques for predicting the phonon-defect scattering rate without fitting parameters. Taking advantage of the extended phonon normal mode analysis, we obtained the spectral phonon relaxation time and mean free path (MFP) in defected graphene and studied the impacts of three common types of defects: Stone-Thrower-Wales (STW) defect, double vacancy (DV), and monovacancy (MV). The phonon-STW defect scattering rate is found to have no significant frequency dependence, and as a result, the relative contribution of long-wavelength phonons sharply decreases. In contrast, the phonon scattering by DVs or MVs exhibits a frequency dependence of τp-d -1˜ω1.1 -1.3 except for a few long-wavelength phonons, revisiting the traditionally used ˜ω4 dependence. We note that although MV-defected graphene has the lowest thermal conductivity as compared to the other two defected graphene samples at the same defect concentration, it has a portion of phonons with the longest MFP. The contribution from the long-MFP and long-wavelength phonons does not decrease much as the vacancy concentration increases. STW defect and MV block more out-of-plane modes than in-plane modes, while DV has less bias for which mode to block. As the MV concentration increases from 0 to 1.1%, the relative contribution from out-of-plane modes decreases from 30% to 18%, while that of the transverse acoustic mode remains at around 30%. These findings of spectral phonon properties can provide more insight than the effective properties and benefit the prospective phononic engineering.
Hannah, Daniel C; Brown, Kristen E; Young, Ryan M; Wasielewski, Michael R; Schatz, George C; Co, Dick T; Schaller, Richard D
2013-09-06
We report femtosecond stimulated Raman spectroscopy measurements of lattice dynamics in semiconductor nanocrystals and characterize longitudinal optical (LO) phonon production during confinement-enhanced, ultrafast intraband relaxation. Stimulated Raman signals from unexcited CdSe nanocrystals produce a spectral shape similar to spontaneous Raman signals. Upon photoexcitation, stimulated Raman amplitude decreases owing to experimentally resolved ultrafast phonon generation rates within the lattice. We find a ∼600 fs, particle-size-independent depletion time attributed to hole cooling, evidence of LO-to-acoustic down-conversion, and LO phonon mode softening.
Zhou, Yanguang; Zhang, Xiaoliang; Hu, Ming
2017-02-08
By carefully and systematically performing Green-Kubo equilibrium molecular dynamics simulations, we report that the thermal conductivity (κ) of Si nanowires (NWs) does not diverge but converges and increases steeply when NW diameter (D) becomes extremely small (dκ/dD < 0), a long debate of one-dimensional heat conduction in history. The κ of the thinnest possible Si NWs reaches a superhigh level that is as large as more than 1 order of magnitude higher than its bulk counterpart. The abnormality is explained in terms of the dominant normal (N) process (energy and momentum conservation) of low frequency acoustic phonons that induces hydrodynamic phonon flow in the Si NWs without being scattered. With D increasing, the downward shift of optical phonons triggers strong Umklapp (U) scattering with acoustic phonons and attenuates the N process, leading to the regime of phonon boundary scattering (dκ/dD < 0). The two competing mechanisms result in nonmonotonic diameter dependence of κ with minima at critical diameter of 2-3 nm. Our results unambiguously demonstrate the converged κ and the clear trend of κ ∼ D for extremely thin Si NWs by fully elucidating the competition between the hydrodynamic phonon flow and phonon boundary scattering.
Phonons in active microfluidic crystals
NASA Astrophysics Data System (ADS)
Tsang, Alan Cheng Hou; Kanso, Eva
2016-11-01
One-dimensional crystals of driven particles confined in quasi two-dimensional microfluidic channels have been shown to exhibit propagating sound waves in the form of 'phonons', including both transverse and longitudinal normal modes. Here, we focus on one-dimensional crystals of motile particles in uniform external flows. We study the propagation of phonons in the context of an idealized model that accounts for hydrodynamic interactions among the motile particles. We obtain a closed-form analytical expression for the dispersion relation of the phonons. In the moving frame of reference of the crystals, the traveling directions of the phonons depend on the intensity of the external flow, and are exactly opposite for the transverse and longitudinal modes. We further investigate the stability of the phonons and show that the longitudinal mode is linearly stable, whereas the transverse mode is subject to an instability arising from the activity and orientation dynamics of the motile particles. These findings are important for understanding the propagation of disturbances and instabilities in confined motile particles, and could generate practical insights into the transport of motile cells in microfluidic devices.
Band structures in the nematic elastomers phononic crystals
NASA Astrophysics Data System (ADS)
Yang, Shuai; Liu, Ying; Liang, Tianshu
2017-02-01
As one kind of new intelligent materials, nematic elastomers (NEs) represent an exciting physical system that combines the local orientational symmetry breaking and the entropic rubber elasticity, producing a number of unique physical phenomena. In this paper, the potential application of NEs in the band tuning is explored. The band structures in two kinds of NE phononic crystals (PCs) are investigated. Through changing NE intrinsic parameters, the influence of the porosity, director rotation and relaxation on the band structures in NE PCs are analyzed. This work is a meaningful try for application of NEs in acoustic field and proposes a new intelligent strategy in band turning.
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Theory of low-power ultra-broadband terahertz sideband generation in bi-layer graphene
NASA Astrophysics Data System (ADS)
Crosse, J. A.; Xu, Xiaodong; Sherwin, Mark S.; Liu, R. B.
2014-09-01
In a semiconductor illuminated by a strong terahertz (THz) field, optically excited electron-hole pairs can recombine to emit light in a broad frequency comb evenly spaced by twice the THz frequency. Such high-order THz sideband generation is of interest both as an example of extreme nonlinear optics and also as a method for ultrafast electro-optical modulation. So far, this phenomenon has only been observed with large field strengths (~10 kV cm-1), an obstacle for technological applications. Here we predict that bi-layer graphene generates high-order sidebands at much weaker THz fields. We find that a THz field of strength 1 kV cm-1 can produce a high-sideband spectrum of about 30 THz, 100 times broader than in GaAs. The sidebands are generated despite the absence of classical collisions, with the quantum coherence of the electron-hole pairs enabling recombination. These remarkable features lower the barrier to desktop electro-optical modulation at THz frequencies, facilitating ultrafast optical communications.
Observation of Synchrotron Sidebands in a Storage-Ring-Based Seeded Free-Electron Laser
Labat, M.; Hosaka, M.; Yamamoto, N.; Shimada, M.; Katoh, M.; Couprie, M. E.
2009-01-09
Seeded free-electron lasers (FELs) are among the future fourth-generation light sources in the vacuum ultraviolet and x-ray spectral regions. We analyze the seed temporal coherence preservation in the case of coherent harmonic generation FELs, including spectral narrowing and structure degradation. Indeed, the electron synchrotron motion driven by the seeding laser can cause sideband growth in the FEL spectrum.
High-accurate optical vector analysis based on optical single-sideband modulation
NASA Astrophysics Data System (ADS)
Xue, Min; Pan, Shilong
2016-11-01
Most of the efforts devoted to the area of optical communications were on the improvement of the optical spectral efficiency. Varies innovative optical devices are thus developed to finely manipulate the optical spectrum. Knowing the spectral responses of these devices, including the magnitude, phase and polarization responses, is of great importance for their fabrication and application. To achieve high-resolution characterization, optical vector analyzers (OVAs) based on optical single-sideband (OSSB) modulation have been proposed and developed. Benefiting from the mature and highresolution microwave technologies, the OSSB-based OVA can potentially achieve a resolution of sub-Hz. However, the accuracy is restricted by the measurement errors induced by the unwanted first-order sideband and the high-order sidebands in the OSSB signal, since electrical-to-optical conversion and optical-to-electrical conversion are essentially required to achieve high-resolution frequency sweeping and extract the magnitude and phase information in the electrical domain. Recently, great efforts have been devoted to improve the accuracy of the OSSB-based OVA. In this paper, the influence of the unwanted-sideband induced measurement errors and techniques for implementing high-accurate OSSB-based OVAs are discussed.
Single-sideband modulator accurately reproduces phase information in 2-Mc signals
NASA Technical Reports Server (NTRS)
Strenglein, H. F.
1966-01-01
Phase-locked oscillator system employing solid state components acts as a single-sideband modulator to accurately reproduce phase information in 2-Mc signals. This system is useful in telemetry, aircraft communications and position-finding stations, and VHF test circuitry.
Coulomb-interaction-dependent effect of high-order sideband generation in an optomechanical system
NASA Astrophysics Data System (ADS)
Kong, Cui; Xiong, Hao; Wu, Ying
2017-03-01
High-order sideband generation in an optomechanical system coupled to a charged object is discussed, and the features of Coulomb-interaction-dependent effect are identified. We show that the Coulomb-interaction-dependent effect of high-order sideband generation exhibits essential difference between the case of weak control field and strong control field. In the weak control field case, the output spectra are in the perturbative regime and there is hardly any Coulomb-interaction-dependent effect in an optomechanical system coupling to an object with a small amount of charge. In the strong control field case, the output spectra are in the nonperturbative regime and robust Coulomb-interaction-dependent effect arises even if there are few charges. The amplitudes of specific sidebands are also discussed, and it is shown that Coulomb interaction plays an important role in achieving optomechanical control. Due to the extremely sensitive charge number, the Coulomb-interaction-dependent effect of high-order sideband generation is remarkable in many aspects and may be used to precision measurement of electrical charges beyond the linearized optomechanical interaction.
Design Of Dual Polarisation Sideband Separation Mixer For ALMA Band 5
NASA Astrophysics Data System (ADS)
Billade, Bhushan
2009-09-01
This licentiate is focused on the design and development of Superconductor-Insulator-Superconductor (SIS) junction mixer for ALMA Band 5, one of the ten frequency bands of the Atacama Large Millimeter Array (ALMA) project. ALMA Band 5 is a dual polarisation sideband separation heterodyne receiver covering radio frequencies (RF) from 163 GHz to 211 GHz, with 4-8 GHz intermediate frequency (IF). Amongst the other ALMA bands, Band 5 is the lowest frequency band, which uses all-cold optics. That puts strong constrains on the dimensions of all the receiver components. For the SIS mixer, we employ a MMIC-like approach where most of the DSB mixer components, including LO injection circuitry with novel directional coupler, are integrated on the same crystal quartz substrate. The mixer uses a lumped filter technique to extract the IF frequencies, which is non-traditional for SIS mixers. A custom made superconducting Lange coupler with suspended air bridges to connect the fingers of Lange coupler is used. Experimental measurements of the double sideband mixer show state of the art performance with the receiver noise temperature below 30 Kelvin across the entire band. The noise temperature for sideband separation mixer is below 60 Kelvin with sideband rejection better than 12 dB over most of the band.
Saturation of a toroidal Alfvén eigenmode due to enhanced damping of nonlinear sidebands
NASA Astrophysics Data System (ADS)
Todo, Y.; Berk, H. L.; Breizman, B. N.
2012-09-01
This paper examines nonlinear magneto-hydrodynamic effects on the energetic particle driven toroidal Alfvén eigenmode (TAE) for lower dissipation coefficients and with higher numerical resolution than in the previous simulations (Todo et al 2010 Nucl. Fusion 50 084016). The investigation is focused on a TAE mode with toroidal mode number n = 4. It is demonstrated that the mechanism of mode saturation involves generation of zonal (n = 0) and higher-n (n ⩾ 8) sidebands, and that the sidebands effectively increase the mode damping rate via continuum damping. The n = 0 sideband includes the zonal flow peaks at the TAE gap locations. It is also found that the n = 0 poloidal flow represents a balance between the nonlinear driving force from the n = 4 components and the equilibrium plasma response to the n = 0 fluctuations. The spatial profile of the n = 8 sideband peaks at the n = 8 Alfvén continuum, indicating enhanced dissipation due to continuum damping.
Development of digital sideband separating down-conversion for Yuan-Tseh Lee Array
NASA Astrophysics Data System (ADS)
Li, Chao-Te; Kubo, Derek; Cheng, Jen-Chieh; Kuroda, John; Srinivasan, Ranjani; Ho, Solomon; Guzzino, Kim; Chen, Ming-Tang
2016-07-01
This report presents a down-conversion method involving digital sideband separation for the Yuan-Tseh Lee Array (YTLA) to double the processing bandwidth. The receiver consists of a MMIC HEMT LNA front end operating at a wavelength of 3 mm, and sub-harmonic mixers that output signals at intermediate frequencies (IFs) of 2-18 GHz. The sideband separation scheme involves an analog 90° hybrid followed by two mixers that provide down-conversion of the IF signal to a pair of in-phase (I) and quadrature (Q) signals in baseband. The I and Q baseband signals are digitized using 5 Giga sample per second (Gsps) analog-to-digital converters (ADCs). A second hybrid is digitally implemented using field-programmable gate arrays (FPGAs) to produce two sidebands, each with a bandwidth of 1.6 GHz. The 2 x 1.6 GHz band can be tuned to cover any 3.6 GHz window within the aforementioned IF range of the array. Sideband rejection ratios (SRRs) above 20 dB can be obtained across the 3.6 GHz bandwidth by equalizing the power and delay between the I and Q baseband signals. Furthermore, SRRs above 30 dB can be achieved when calibration is applied.
Strain induced modification in phonon dispersion curves of monolayer boron pnictides
Jha, Prafulla K. E-mail: prafullaj@yahoo.com; Soni, Himadri R.
2014-01-14
In the frame work of density functional theory, the biaxial strain induced phonon dispersion curves of monolayer boron pnictides (BX, X = N, P, As, and Sb) have been investigated. The electron-ion interactions have been modelled using ultrasoft pseudopotentials while exchange-correlation energies have been approximated by the method of local density approximation in the parameterization of Perdew-Zunger. The longitudinal and transverse acoustic phonon modes of boron pnictide sheets show linear dependency on wave vector k{sup →} while out of plane mode varies as k{sup 2}. The in-plane longitudinal and out of plane transverse optical modes in boron nitride displaying significant dispersion similar to graphene. We have analyzed the biaxial strain dependent behaviour of out of plane acoustic phonon mode which is linked to ripple for four BX sheets using a model equation with shell elasticity theory. The strain induces the hardening of this mode with tendency to become more linear with increase in strain percentage. The strain induced hardening of out of plane acoustic phonon mode indicates the absence of rippling in these compounds. Our band structure calculations for both unstrained and strained 2D h-BX are consistent with previous calculations.
Phonon dynamics of americium telluride
NASA Astrophysics Data System (ADS)
Arya, B. S.; Aynyas, Mahendra; Ahirwar, Ashok K.; Sanyal, S. P.
2013-06-01
We report for the first time the complete phonon dispersion curves for Americium telluride (AmTe) using a breathing shell models (BSM) to establish their predominant ionic nature. The results obtained in the present study show the general features of the phonon spectrum. We could not compare our results with the experimental measurements as they are not available so far. We emphasize the need of neutron scattering measurements to compare our results. We also report, for the first time specific heat for this compound.
Scattering of phonons by vacancies
Ratsifaritana, C.A.; Klemens, P.G.
1987-11-01
The scattering of phonons by vacancies is estimated by a perturbation technique in terms of the missing mass and the missing linkages. An argument is given why distortion effects can be disregarded. The resonance frequency of the defect is sufficiently high so that resonance effects can be disregarded for phonons in the important frequency range for thermal conduction. The theory is applied to the thermal resistance by vacancies in cases where the vacancy concentration is known: potassium chloride with divalent cations, nonstoichiometric zirconium carbide, and tin telluride.
Generation and detection of incoherent phonons in picosecond ultrasonics.
Perrin, B; Péronne, E; Belliard, L
2006-12-22
In picosecond ultrasonics experiments the absorption of a femtosecond laser pulse in a thin metallic transducer is used to generate very short acoustic pulses. These pulses are made of coherent longitudinal waves with a frequency spectrum that can reach 100-200 GHz. The laser pulse absorption gives rise to a heating of the film of a few Kelvin within a typical time of 1 ps. Later on, the heat goes in the substrate through an interface thermal resistance and is diffused by thermal conduction. At very low temperature and in pure crystals the thermal phonons emitted by the heated metallic film can propagate ballistically over large distances and produce a so-called heat pulse. We report on the experimental evidence of the coexistence of the coherent acoustic pulse and the incoherent heat pulse generated and detected by laser ultrasonics.
Modulations of thermal properties of graphene by strain-induced phonon engineering
NASA Astrophysics Data System (ADS)
Tada, Kento; Funatani, Takashi; Konabe, Satoru; Sasaoka, Kenji; Ogawa, Matsuto; Souma, Satofumi; Yamamoto, Takahiro
2017-02-01
Modulation of the thermal properties of graphene due to strain-induced phononic band engineering was theoretically investigated by first-principles calculations based on the density functional theory. The high-energy phonon modes are found to exhibit softening owing to the strain, whereas a low-energy acoustic mode (out-of-plane mode) exhibits hardening. Moreover, the dispersion relation of the out-of-plane mode associated with the strain essentially changes from quadratic (∝ k 2) to linear (∝ k). Accordingly, the temperature dependence of the low-temperature specific heat also changes from linear (∝ T) to quadratic (∝ T 2).
The effects of substrate phonon mode scattering on transport in carbon nanotubes.
Perebeinos, Vasili; Rotkin, Slava V; Petrov, Alexey G; Avouris, Phaedon
2009-01-01
Carbon nanotubes (CNTs) have large intrinsic carrier mobility due to weak acoustic phonon scattering. However, unlike two-dimensional metal-oxide-semiconductor field effect transistors (MOSFETs), substrate surface polar phonon (SPP) scattering has a dramatic effect on the CNTFET mobility, due to the reduced vertical dimensions of the latter. We find that for the van der Waals distance between CNT and an SiO2 substrate, the low-field mobility at room temperature is reduced by almost an order of magnitude depending on the tube diameter. We predict additional experimental signatures of the SPP mechanism in dependence of the mobility on density, temperature, tube diameter, and CNT-substrate separation.
Current & Heat Transport in Graphene Nanoribbons: Role of Non-Equilibrium Phonons
NASA Astrophysics Data System (ADS)
Pennington, Gary; Finkenstadt, Daniel
2010-03-01
The conducting channel of a graphitic nanoscale device is expected to experience a larger degree of thermal isolation when compared to traditional inversion channels of electronic devices. This leads to enhanced non-equilibrium phonon populations which are likely to adversely affect the mobility of graphene-based nanoribbons due to enhanced phonon scattering. Recent reports indicating the importance of carrier scattering with substrate surface polar optical phonons in carbon nanotubes^1 and graphene^2,3 show that this mechanism may allow enhanced heat removal from the nanoribbon channel. To investigate the effects of hot phonon populations on current and heat conduction, we solve the graphene nanoribbon multiband Boltzmann transport equation. Monte Carlo transport techniques are used since phonon populations may be tracked and updated temporally.^4 The electronic structure is solved using the NRL Tight-Binding method,^5 where carriers are scattered by confined acoustic, optical, edge and substrate polar optical phonons. [1] S. V. Rotkin et al., Nano Lett. 9, 1850 (2009). [2] J. H. Chen, C. Jang, S. Xiao, M. Ishigami and M. S. Fuhrer, Nature Nanotech. 3, 206 (2008). [3] V. Perebeinos and P. Avouris, arXiv:0910.4665v1 [cond-mat.mes-hall] (2009). [4] P. Lugli et al., Appl. Phys. Lett. 50, 1251 (1987). [5] D. Finkenstadt, G. Pennington & M.J. Mehl, Phys. Rev. B 76, 121405(R) (2007).
Low temperature phonon-drag thermopower in a monolayer MoS{sub 2}
Bhargavi, K. S. Kubakaddi, S. S.
2015-06-24
Phonon-drag thermopower S{sup g} is studied theoretically in a monolayer MoS{sub 2} as a function of temperature T. Electron-acoustic phonon (el-ap) interaction via deformation potential (DP) coupling of TA (LA) phonons is taken to be unscreened (screened) and piezoelectric (PE) coupling of LA and TA phonons is taken to be screened. S{sup g} due to DP coupling of TA phonons is found to be dominant over all other mechanisms. In the Bloch-Gruneisen (BG) regime power law S{sup g} ∼ T{sup 3} (T {sup 5}) is predicted for unscreened (screened) el-ap interaction a characteristic of two-dimensional phonons with linear dispersion. Screening strongly suppresses S{sup g} due to large effective mass of the electrons. We find that, S{sup g} due to screened DP and PE couplings are nearly same in contrast with the results in GaAs heterojunctions. With the increasing T its exponent decreases and reaches a sublinear value.
Walczak, Kamil; Yerkes, Kirk L.
2014-05-07
We examine heat transport carried by acoustic phonons in the systems composed of nanoscale chains of masses coupled to two thermal baths of different temperatures. Thermal conductance is obtained by using linearized Landauer-type formula for heat flux with phonon transmission probability calculated within atomistic Green's functions (AGF) method. AGF formalism is extended onto dissipative chains of masses with harmonic coupling beyond nearest-neighbor approximation, while atomistic description of heat reservoirs is also included into computational scheme. In particular, the phonon lifetimes and the phonon frequency shifts are discussed for harmonic lattices of different dimensions. Further, resonant structure of phonon transmission spectrum is analyzed with respect to reservoir-induced effects, molecular damping, and mass-to-mass harmonic coupling. Analysis of transmission zeros (antiresonances) and their accompanied Fano-shape resonances are discussed as a result of interference effects between different vibrational modes. Finally, we also predict subdiffusive transport regime for low-frequency ballistic phonons propagated along a linear chain of harmonically coupled masses.
NASA Astrophysics Data System (ADS)
Walczak, Kamil; Yerkes, Kirk L.
2014-05-01
We examine heat transport carried by acoustic phonons in the systems composed of nanoscale chains of masses coupled to two thermal baths of different temperatures. Thermal conductance is obtained by using linearized Landauer-type formula for heat flux with phonon transmission probability calculated within atomistic Green's functions (AGF) method. AGF formalism is extended onto dissipative chains of masses with harmonic coupling beyond nearest-neighbor approximation, while atomistic description of heat reservoirs is also included into computational scheme. In particular, the phonon lifetimes and the phonon frequency shifts are discussed for harmonic lattices of different dimensions. Further, resonant structure of phonon transmission spectrum is analyzed with respect to reservoir-induced effects, molecular damping, and mass-to-mass harmonic coupling. Analysis of transmission zeros (antiresonances) and their accompanied Fano-shape resonances are discussed as a result of interference effects between different vibrational modes. Finally, we also predict subdiffusive transport regime for low-frequency ballistic phonons propagated along a linear chain of harmonically coupled masses.
Marshall, T.C.; Bhattacharjee, A.
1994-10-01
Several studies have been made of optical guiding and sideband effects that might occur using the hardware of certain experiments which are scheduled to operate in late 1994 at the Accelerator Test Facility at Brookhaven. We find that experimental observations of optical guiding and sidebanding would be fruitful in connection with the blue-green FEL oscillator experiment. Should the data bear out our expectations (obtained from TDA code runs described below), then some confidence would be established in our tentative conclusion --based upon the code as well as analytic theory-- that neither optical guiding nor sidebands are to be expected in connection with the IFEL accelerator.
Coherent phonon-grain boundary scattering in silicon inverse opals.
Ma, Jun; Parajuli, Bibek R; Ghossoub, Marc G; Mihi, Agustin; Sadhu, Jyothi; Braun, Paul V; Sinha, Sanjiv
2013-02-13
We report measurements and modeling of thermal conductivity in periodic three-dimensional dielectric nanostructures, silicon inverse opals. Such structures represent a three-dimensional "phononic crystal" but affect heat flow instead of acoustics. Employing the Stober method, we fabricate high quality silica opal templates that on filling with amorphous silicon, etching and recrystallizing produce silicon inverse opals. The periodicities and shell thicknesses are in the range 420-900 and 18-38 nm, respectively. The thermal conductivity of inverse opal films are relatively low, ~0.6-1.4 W/mK at 300 K and arise due to macroscopic bending of heat flow lines in the structure. The corresponding material thermal conductivity is in the range 5-12 W/mK and has an anomalous ~T(1.8) dependence at low temperatures, distinct from the typical ~T(3) behavior of bulk polycrystalline silicon. Using phonon scattering theory, we show such dependence arising from coherent phonon reflections in the intergrain region. This is consistent with an unconfirmed theory proposed in 1955. The low thermal conductivity is significant for applications in photonics where they imply significant temperature rise at relatively low absorption and in thermoelectrics, where they suggest the possibility of enhancement in the figure of merit for polysilicon with optimal doping.
Phonon impedance matching: minimizing interfacial thermal resistance of thin films
NASA Astrophysics Data System (ADS)
Polanco, Carlos; Zhang, Jingjie; Ghosh, Avik
2014-03-01
The challenge to minimize interfacial thermal resistance is to allow a broad band spectrum of phonons, with non-linear dispersion and well defined translational and rotational symmetries, to cross the interface. We explain how to minimize this resistance using a frequency dependent broadening matrix that generalizes the notion of acoustic impedance to the whole phonon spectrum including symmetries. We show how to ``match'' two given materials by joining them with a single atomic layer, with a multilayer material and with a graded superlattice. Atomic layer ``matching'' requires a layer with a mass close to the arithmetic mean (or spring constant close to the harmonic mean) to favor high frequency phonon transmission. For multilayer ``matching,'' we want a material with a broadening close to the geometric mean to maximize transmission peaks. For graded superlattices, a continuous sequence of geometric means translates to an exponentially varying broadening that generates a wide-band antireflection coating for both the coherent and incoherent limits. Our results are supported by ``first principles'' calculations of thermal conductance for GaAs / Gax Al1 - x As / AlAs thin films using the Non-Equilibrium Greens Function formalism coupled with Density Functional Perturbation Theory. NSF-CAREER (QMHP 1028883), NSF-IDR (CBET 1134311), XSEDE.
Otelaja, O. O.; Robinson, R. D.
2015-10-26
In this work, the mechanism for enhanced phonon backscattering in silicon is investigated. An understanding of phonon propagation through substrates has implications for engineering heat flow at the nanoscale, for understanding sources of decoherence in quantum systems, and for realizing efficient phonon-mediated particle detectors. In these systems, phonons that backscatter from the bottom of substrates, within the crystal or from interfaces, often contribute to the overall detector signal. We utilize a microscale phonon spectrometer, comprising superconducting tunnel junction emitters and detectors, to specifically probe phonon backscattering in silicon substrates (∼500 μm thick). By etching phonon “enhancers” or deep trenches (∼90 μm) around the detectors, we show that the backscattered signal level increases by a factor of ∼2 for two enhancers versus one enhancer. Using a geometric analysis of the phonon pathways, we show that the mechanism of the backscattered phonon enhancement is due to confinement of the ballistic phonon pathways and increased scattering off the enhancer walls. Our result is applicable to the geometric design and patterning of substrates that are employed in phonon-mediated detection devices.
Nonlinear acoustic characteristics of Fatigue microcracks in al alloy plate
NASA Astrophysics Data System (ADS)
Gao, G. L.; Li, D. Y.; Shi, D. Q.; Dong, J. W.; Shi, X. D.; Teng, F.
2011-02-01
A system consisting of piezoelectric transducers, arbitrary waveform generator, power amplifier, laser vibrometer, digital oscilloscope, and a computer has been constructed to study the nonlinear acoustic characteristics of fatigue microcracks of 2024-T351 aluminum alloy plates. Using two different frequency signals (fH=810 kHz, fL=100 kHz), the intact and microcracked samples are experimented, respectively. The experimental results show that in the intact samples there are only two fundamental frequencies and no harmonics and sidebands occur. In the microcracked samples, there is an abundance of the harmonics and sidebands, and the frequencies fH±fL and fH±2fL rise. These new frequency components can be used to indicate the presence of a microcrack or damage.
Phononic Crystal Tunable via Ferroelectric Phase Transition
NASA Astrophysics Data System (ADS)
Xu, Chaowei; Cai, Feiyan; Xie, Shuhong; Li, Fei; Sun, Rong; Fu, Xianzhu; Xiong, Rengen; Zhang, Yi; Zheng, Hairong; Li, Jiangyu
2015-09-01
Phononic crystals (PCs) consisting of periodic materials with different acoustic properties have potential applications in functional devices. To realize more smart functions, it is desirable to actively control the properties of PCs on demand, ideally within the same fabricated system. Here, we report a tunable PC made of Ba0.7Sr0.3Ti O3 (BST) ceramics, wherein a 20-K temperature change near room temperature results in a 20% frequency shift in the transmission spectra induced by a ferroelectric phase transition. The tunability phenomenon is attributed to the structure-induced resonant excitation of A0 and A1 Lamb modes that exist intrinsically in the uniform BST plate, while these Lamb modes are sensitive to the elastic properties of the plate and can be modulated by temperature in a BST plate around the Curie temperature. The study finds opportunities for creating tunable PCs and enables smart temperature-tuned devices such as the Lamb wave filter or sensor.
Negative refraction imaging of acoustic metamaterial lens in the supersonic range
Han, Jianning; Wen, Tingdun; Yang, Peng; Zhang, Lu
2014-05-15
Acoustic metamaterials with negative refraction index is the most promising method to overcome the diffraction limit of acoustic imaging to achieve ultrahigh resolution. In this paper, we use localized resonant phononic crystal as the unit cell to construct the acoustic negative refraction lens. Based on the vibration model of the phononic crystal, negative quality parameters of the lens are obtained while excited near the system resonance frequency. Simulation results show that negative refraction of the acoustic lens can be achieved when a sound wave transmiting through the phononic crystal plate. The patterns of the imaging field agree well with that of the incident wave, while the dispersion is very weak. The unit cell size in the simulation is 0.0005 m and the wavelength of the sound source is 0.02 m, from which we show that acoustic signal can be manipulated through structures with dimensions much smaller than the wavelength of incident wave.
Nanoscale control of phonon excitations in graphene
Kim, Hyo Won; Ko, Wonhee; Ku, JiYeon; Jeon, Insu; Kim, Donggyu; Kwon, Hyeokshin; Oh, Youngtek; Ryu, Seunghwa; Kuk, Young; Hwang, Sung Woo; Suh, Hwansoo
2015-01-01
Phonons, which are collective excitations in a lattice of atoms or molecules, play a major role in determining various physical properties of condensed matter, such as thermal and electrical conductivities. In particular, phonons in graphene interact strongly with electrons; however, unlike in usual metals, these interactions between phonons and massless Dirac fermions appear to mirror the rather complicated physics of those between light and relativistic electrons. Therefore, a fundamental understanding of the underlying physics through systematic studies of phonon interactions and excitations in graphene is crucial for realising graphene-based devices. In this study, we demonstrate that the local phonon properties of graphene can be controlled at the nanoscale by tuning the interaction strength between graphene and an underlying Pt substrate. Using scanning probe methods, we determine that the reduced interaction due to embedded Ar atoms facilitates electron–phonon excitations, further influencing phonon-assisted inelastic electron tunnelling. PMID:26109454
Microfabricated bulk wave acoustic bandgap device
Olsson, Roy H.; El-Kady, Ihab F.; McCormick, Frederick; Fleming, James G.; Fleming, Carol
2010-06-08
A microfabricated bulk wave acoustic bandgap device comprises a periodic two-dimensional array of scatterers embedded within the matrix material membrane, wherein the scatterer material has a density and/or elastic constant that is different than the matrix material and wherein the periodicity of the array causes destructive interference of the acoustic wave within an acoustic bandgap. The membrane can be suspended above a substrate by an air or vacuum gap to provide acoustic isolation from the substrate. The device can be fabricated using microelectromechanical systems (MEMS) technologies. Such microfabricated bulk wave phononic bandgap devices are useful for acoustic isolation in the ultrasonic, VHF, or UHF regime (i.e., frequencies of order 1 MHz to 10 GHz and higher, and lattice constants of order 100 .mu.m or less).
Microfabricated bulk wave acoustic bandgap device
Olsson, Roy H.; El-Kady, Ihab F.; McCormick, Frederick; Fleming, James G.; Fleming, legal representative, Carol
2010-11-23
A microfabricated bulk wave acoustic bandgap device comprises a periodic two-dimensional array of scatterers embedded within the matrix material membrane, wherein the scatterer material has a density and/or elastic constant that is different than the matrix material and wherein the periodicity of the array causes destructive interference of the acoustic wave within an acoustic bandgap. The membrane can be suspended above a substrate by an air or vacuum gap to provide acoustic isolation from the substrate. The device can be fabricated using microelectromechanical systems (MEMS) technologies. Such microfabricated bulk wave phononic bandgap devices are useful for acoustic isolation in the ultrasonic, VHF, or UHF regime (i.e., frequencies of order 1 MHz to 10 GHz and higher, and lattice constants of order 100 .mu.m or less).
NASA Astrophysics Data System (ADS)
Luo, Yixiu; Wang, Jiemin; Li, Yiran; Wang, Jingyang
2016-07-01
Modification of lattice thermal conductivity (κL) of a solid by means of hydrostatic pressure (P) has been a crucially interesting approach that targets a broad range of advanced materials from thermoelectrics and thermal insulators to minerals in mantle. Although it is well documented knowledge that thermal conductivity of bulk materials normally increase upon hydrostatic pressure, such positive relationship is seriously challenged when it comes to ceramics with complex crystal structure and heterogeneous chemical bonds. In this paper, we predict an abnormally negative trend dκL/dP < 0 in Y2Si2O7 silicate using density functional theoretical calculations. The mechanism is disclosed as combined effects of slightly decreased group velocity and significantly augmented scattering of heat-carrying acoustic phonons in pressured lattice, which is originated from pressure-induced downward shift of low-lying optic and acoustic phonons. The structural origin of low-lying optic phonons as well as the induced phonon anharmonicity is also qualitatively elucidated with respect to intrinsic bonding heterogeneity of Y2Si2O7. The present results are expected to bring deeper insights for phonon engineering and modulation of thermal conductivity in complex solids with diverging structural flexibility, enormous bonding heterogeneity, and giant phonon anharmonicity.
Luo, Yixiu; Wang, Jiemin; Li, Yiran; Wang, Jingyang
2016-01-01
Modification of lattice thermal conductivity (κL) of a solid by means of hydrostatic pressure (P) has been a crucially interesting approach that targets a broad range of advanced materials from thermoelectrics and thermal insulators to minerals in mantle. Although it is well documented knowledge that thermal conductivity of bulk materials normally increase upon hydrostatic pressure, such positive relationship is seriously challenged when it comes to ceramics with complex crystal structure and heterogeneous chemical bonds. In this paper, we predict an abnormally negative trend dκL/dP < 0 in Y2Si2O7 silicate using density functional theoretical calculations. The mechanism is disclosed as combined effects of slightly decreased group velocity and significantly augmented scattering of heat-carrying acoustic phonons in pressured lattice, which is originated from pressure-induced downward shift of low-lying optic and acoustic phonons. The structural origin of low-lying optic phonons as well as the induced phonon anharmonicity is also qualitatively elucidated with respect to intrinsic bonding heterogeneity of Y2Si2O7. The present results are expected to bring deeper insights for phonon engineering and modulation of thermal conductivity in complex solids with diverging structural flexibility, enormous bonding heterogeneity, and giant phonon anharmonicity. PMID:27430670
Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe1-xMxSi, M=Ir,Os
Delaire, O.; Al-Qasir, Iyad I.; May, Andrew F.; ...
2015-03-31
The vibrational behavior of heavy substitutional impurities (M=Ir,Os) in Fe1-xMxSi (x = 0, 0.02, 0.04, 0.1) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. In this paper, our INS measurements on single-crystals mapped the four-dimensional dynamical structure factor, S(Q;E), for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers and increases electron-phonon coupling, leads tomore » softened interatomic force-constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S(Q,E) from INS through a Green's function model incorporating the phonon self-energy based on first-principles density functional theory (DFT) simulations. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Finally, our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.« less
Energy loss to intravalley acoustic modes in nano-dimensional wire structures at low temperatures
NASA Astrophysics Data System (ADS)
Nag, S.; Das, B.; Basu, A.; Das, J.; Bhattacharya, D. P.; Sarkar, C. K.
2017-03-01
The theory of rate of loss of energy of non-equilibrium electrons due to inelastic interaction with the intravalley acoustic phonons in a nano-dimensional semiconductor wire has been developed under the condition of low lattice temperature, when the approximations of the well known traditional theory are not valid. Numerical results are obtained for narrow-channel GaAs-GaAlAs wires structures. On comparison with other available results it is revealed that the finite energy of the intravalley acoustic phonons and, the use of the full form of the phonon distribution without truncation to the equipartition law, produce significant changes in the energy loss characteristics at low temperatures.
Sotnikov, V.I.; Fiala, V.; Lefeuvre, F.; Lagoutte, D. ); Mogilevsky, M. )
1991-07-01
Symmetric sidebands are observed in the ionosphere by the AUREOL 3 satellite when it passes at a height of 1,200 km above the VLF transmitter at the Komsomolsk-on-Amur Alpha station (50{degree}5 N, 135{degree} E, frequency 11.90 and 12.65 kHz). The sidebands are about 500 Hz off the carrier frequency of Alpha pulses. They are approximately 20 dB lower than the transmitter signal, and they appear only when ELF natural emission above the local proton gyrofrequency is observed. The data are presented and analyzed. The nonlinear coupling of the VLF transmitter signal to natural ELF emission is invoked to explain the symmetric sidebands. It is shown that the nonlinear current excited by the beats of VLF and ELF waves is strong enough to explain the sideband amplitude.
Phonon assisted resonant tunneling and its phonons control
NASA Astrophysics Data System (ADS)
Kusmartsev, F. V.; Krevchik, V. D.; Semenov, M. B.; Filatov, D. O.; Shorokhov, A. V.; Bukharaev, A. A.; Dakhnovsky, Y.; Nikolaev, A. V.; Pyataev, N. A.; Zaytsev, R. V.; Krevchik, P. V.; Egorov, I. A.; Yamamoto, K.; Aringazin, A. K.
2016-09-01
We observe a series of sharp resonant features in the tunneling differential conductance of InAs quantum dots. We found that dissipative quantum tunneling has a strong influence on the operation of nanodevices. Because of such tunneling the current-voltage characteristics of tunnel contact created between atomic force microscope tip and a surface of InAs/GaAs quantum dots display many interesting peaks. We found that the number, position, and heights of these peaks are associated with the phonon modes involved. To describe the found effect we use a quasi-classical approximation. There the tunneling current is related to a creation of a dilute instanton-anti-instanton gas. Our experimental data are well described with exactly solvable model where one charged particle is weakly interacting with two promoting phonon modes associated with external medium. We conclude that the characteristics of the tunnel nanoelectronic devices can thus be controlled by a proper choice of phonons existing in materials, which are involved.
Microwave sidebands for laser cooling by direct modulation of a tapered amplifier
NASA Astrophysics Data System (ADS)
Mahnke, J.; Kulas, S.; Geisel, I.; Jöllenbeck, S.; Ertmer, W.; Klempt, C.
2013-06-01
Laser cooling of atoms usually necessitates several laser frequencies. Alkaline atoms, for example, are cooled by two lasers with a frequency difference in the gigahertz range. This gap cannot be closed with simple shifting techniques. Here, we present a method of generating sidebands at 6.6 GHz by modulating the current of a tapered amplifier, which is seeded by an unmodulated master laser. The sidebands enable trapping of 1.1 × 109 87Rb atoms in a chip-based magneto-optical trap. Compared to the direct modulation of the master laser, this method allows for an easy implementation, a fast adjustment over a wide frequency range, and the simultaneous extraction of unmodulated light for manipulation and detection. The low power consumption, small size, and applicability for multiple frequencies benefit a wide range of applications reaching from atom-based mobile sensors to the laser cooling of molecules.
Design and performance of mass-produced sideband separating SIS mixers for ALMA band 4 receivers
NASA Astrophysics Data System (ADS)
Kojima, Takafumi; Kuroiwa, Koichi; Takahashi, Toshikazu; Fujii, Yumi; Uzawa, Yoshinori; Asayama, Shin'ichiro; Noguchi, Takashi
2015-09-01
We have designed and mass-produced low-noise sideband separating superconductor-insulator-superconductor (SIS) mixers for the Atacama Large Millimeter/submillimeter Array (ALMA) band 4 over the frequency range of 125-163 GHz. An integrated design was adopted for the band 4 sideband separating (2SB) mixer block because of the advantages it offers in terms of compactness, reduced testing time and lower cost. The mixer chip was designed to be robust for handling errors to avoid performance degradation caused by generation of the higher order mode in the mixer chip slot. Detailed analyses revealed its robustness and ability to ensure mass production of the 2SB mixers. Using the robust mixer design in addition to well-established waveguide technologies, all of the 2SB mixers met ALMA specifications for noise temperature and image rejection ratio.
Differential Brillouin fiber sensor based on phase difference on double-sideband pump wave
NASA Astrophysics Data System (ADS)
Lin, Wenqiao; Hong, Xiaobin; Yang, Zhisheng; Wu, Jian; Lin, Jintong
2015-06-01
A configuration based on phase difference on a double-sideband pump wave is proposed to detect the differential variation of temperature or strain in single-mode optical fibers. In our configuration, a probe wave only experiences a differential Brillouin gain contributed by the perturbation of temperature or strain in the sensing fiber. As a result, the power limitation of the probe wave can be alleviated and the photodetector in our configuration does not easily become saturated in the case of a longer sensing range. The spatial resolution is determined by the duration of the phase difference on the two sidebands and the signal-to-noise of our system is nearly twice as high as that of a differential pulse-width pair Brillouin optical time domain analysis sensor since a π-phase shift on the pump wave is employed. The properties and performances of our method are also theoretically derived and experimentally validated.
Dual-Polarization, Sideband-Separating, Balanced Receiver for 1.5 THz
NASA Technical Reports Server (NTRS)
Chattopadhyay, Goutman; Ward, John; Manohara, Harish; Siegel, Peter
2009-01-01
A proposed heterodyne receiver would be capable of detecting electromagnetic radiation in both of two orthogonal linear polarizations, separating sidebands, and providing balanced outputs in a frequency band centered at 1.5 THz with a fractional bandwidth greater than 40 percent. Dual polarization, sideband-separating, and balanced-output receivers are well-known and have been used extensively at frequencies up to about 100 GHz; and there was an earlier proposal for such a receiver for frequencies up to 900 GHz. However, the present proposal represents the first realistic design concept for such a receiver capable of operating above 1 THz. The proposed receiver is intended to be a prototype of mass-producible receiver units, operating at frequencies up to 6 THz, that would be incorporated into highly sensitive heterodyne array instruments to be used in astronomical spectroscopic and imaging studies.
Jeong, Hyun-Woo; Lim, Jae-Guyn; Kim, Hyung-Jin; Chung, Wonzoo; Kim, Beop-Min
2012-12-01
In order to achieve computationally efficient mirror image rejection during the off-pivot, full-range approach in spectral-domain optical coherence tomography, we used a vestigial sideband (VSB) filter in place of a Hilbert transform. The appropriate choice of the VSB filter parameters enabled almost complete removal of one sideband with much reduced computational load. To determine the optimal filter parameters, we acquired images of the infrared card and analyzed the mirror suppression ratio of the card surface. Comparison between images obtained using the two filters revealed that the computational load is reduced by 52.4±0.17% when using the VSB filter as it requires a much shorter truncation length. Finally, we present the anterior segment images of a human volunteer's eye processed using the VSB filter.
Ab initio study of phonon-induced dephasing of plasmon excitations in silver quantum dots
NASA Astrophysics Data System (ADS)
Guo, Zhenyu; Habenicht, Bradley F.; Liang, Wan-Zhen; Prezhdo, Oleg V.
2010-03-01
Phonon-induced pure dephasing of electronic excitations in silver quantum dots (QDs) is investigated with ab initio molecular dynamics at ambient and low temperatures. Three types of electronic states are studied corresponding to bulk, surface, and plasmon excitations. The electron-phonon coupling is strongest for bulk states and decreases for surface and plasmon states. The plasmon states dephase within 30-40 fs, which is consistent with the recent experiments [M. Z. Liu, M. Pelton, and P. Guyot-Sionnest, Phys. Rev. B 79, 035418 (2009)]. The dephasing time shows weak dependence on the QD size but changes significantly with temperature. The bulk, surface, and plasmon states couple primarily to low-frequency acoustic phonons.
Thermal conductivity in large-J two-dimensional antiferromagnets: Role of phonon scattering
Chernyshev, A. L.; Brenig, Wolfram
2015-08-05
Different types of relaxation processes for magnon heat current are discussed, with a particular focus on coupling to three-dimensional phonons. There is thermal conductivity by these in-plane magnetic excitations using two distinct techniques: Boltzmann formalism within the relaxation-time approximation and memory-function approach. Also considered are the scattering of magnons by both acoustic and optical branches of phonons. We demonstrate an accord between the two methods, regarding the asymptotic behavior of the effective relaxation rates. It is strongly suggested that scattering from optical or zone-boundary phonons is important for magnon heat current relaxation in a high-temperature window of ΘD≲T<< J.
Amplitude-dependent phononic processes in a diatomic granular chain in the weakly nonlinear regime.
Cabaret, Jérémy; Tournat, Vincent; Béquin, Philippe
2012-10-01
Nonlinear acoustic processes of second harmonic generation and nonlinear resonances in a diatomic granular chain (a granular phononic crystal) with static precompression are reported. The observed nonlinear self-action process which manifests itself as shifts in resonance frequencies of the chain leads to amplitude-dependent band edges: the properties of the phononic crystal change as a function of wave amplitude. Observed nonlinear effects at the band edges are exceptionally strong (self-induced attenuation and self-induced transparency) due to the peculiar frequency dependence of the attenuation in these frequency regions. The reported effects open the way for applications in wave tailoring by nonlinear phononic crystals, using amplitude-dependent processes, such as passive amplitude-dependent attenuators or amplifiers and various logical elements.
Biexciton decay and multimagnon sideband in emission spectra of CsMnF 3
NASA Astrophysics Data System (ADS)
Yamaguchi, Y.; Hirano, M.
1980-11-01
Emission spectra of intrinsic and impurity-trapped excitons and their side- bands have been measured in CsMnF 3 by a polarized time-resolved spectroscopy. From a biexcitonic decay of an emission an exciton- exciton interaction was found to be very small in contrast with those of MnF 2 and KMnF 3. Multimagnon sidebands have been assigned with the aid of calculation of magnon density of states.
Double sideband suppressed carrier modulation for stable fiber delivery of radio frequency standards
NASA Astrophysics Data System (ADS)
Nikas, Thomas; Bogris, Adonis; Syvridis, Dimitris
2017-01-01
We theoretically and experimentally investigate the properties of a double sideband suppressed carrier modulation transmission scheme for long distance microwave frequency standard dissemination. The proposed method effectively doubles the transmitted frequency obtaining enhanced phase noise and stability performance. Suppressing the optical carrier also eliminates the dispersion induced signal fading. Important transmission parameters like optical modulation depth and linearity are also improved. Allan deviation and phase noise measurements prove the superior performance of the proposed modulation format.
Long-range distributed Brillouin fiber sensors by use of an unbalanced double sideband probe.
Bernini, Romeo; Minardo, Aldo; Zeni, Luigi
2011-11-21
We propose and demonstrate a long-range Brillouin Optical Time-Domain Analysis (BOTDA) distributed sensing system making use of an unbalanced double sideband probe formed by a Stokes and an anti-Stokes line. In particular, we show that for each measuring condition an optimal Stokes /anti-Stokes input power ratio exists, allowing a larger suppression of nonlocal effects induced by pump depletion. Experiments on a 50 km single-mode sensing fiber with 5 meters spatial resolution are reported.
The Experimental plan of the 4m Resonant Sideband Extraction Prototype for The LCGT
NASA Astrophysics Data System (ADS)
Kawazoe, F.; Kokeyama, K.; Sato, S.; Miyakawa, O.; Somiya, K.; Fukushima, M.; Arai, N.; Kawamura, S.; Sugamoto, A.
2006-03-01
The 4m Resonant Sideband Extraction (RSE) interferometer is a planned prototype of the LCGT interferometer. The aim of the experiment is to operate a powerrecycled Broadband RSE interferometer with suspended optics and to achieve diagonalization of length signals of the central part of the interferometer directly through the optical setup. Details of the 4m RSE interferometer control method as well as the design of the experimental setup will be presented.
Inelastic x-ray scattering measurements of phonon dispersion and lifetimes in PbTe1-x Se x alloys
NASA Astrophysics Data System (ADS)
Tian, Zhiting; Li, Mingda; Ren, Zhensong; Ma, Hao; Alatas, Ahmet; Wilson, Stephen D.; Li, Ju
2015-09-01
PbTe1-x Se x alloys are of special interest to thermoelectric applications. Inelastic x-ray scattering determination of phonon dispersion and lifetimes along the high symmetry directions for PbTe1-x Se x alloys are presented. By comparing with calculated results based on the virtual crystal model calculations combined with ab initio density functional theory, the validity of virtual crystal model is evaluated. The results indicate that the virtual crystal model is overall a good assumption for phonon frequencies and group velocities despite the softening of transverse acoustic phonon modes along [1 1 1] direction, while the treatment of lifetimes warrants caution. In addition, phonons remain a good description of vibrational modes in PbTe1-x Se x alloys.
Inelastic x-ray scattering measurements of phonon dispersion and lifetimes in PbTe1-x Se x alloys.
Tian, Zhiting; Li, Mingda; Ren, Zhensong; Ma, Hao; Alatas, Ahmet; Wilson, Stephen D; Li, Ju
2015-09-23
PbTe1-x Se x alloys are of special interest to thermoelectric applications. Inelastic x-ray scattering determination of phonon dispersion and lifetimes along the high symmetry directions for PbTe1-x Se x alloys are presented. By comparing with calculated results based on the virtual crystal model calculations combined with ab initio density functional theory, the validity of virtual crystal model is evaluated. The results indicate that the virtual crystal model is overall a good assumption for phonon frequencies and group velocities despite the softening of transverse acoustic phonon modes along [1 1 1] direction, while the treatment of lifetimes warrants caution. In addition, phonons remain a good description of vibrational modes in PbTe1-x Se x alloys.
ZUDOV,M.A.; PONOMAREV,I.V.; EFROS,A.L.; DU,R.R.; SIMMONS,JERRY A.; RENO,JOHN L.
2000-05-11
The authors report a new type of oscillations in magnetoresistance observed in high-mobility two-dimensional electron gas (2DEG), in GaAs-AIGaAs heterostructures. Being periodic in 1/B these oscillations appear in weak magnetic field (B < 0.3 T) and only in a narrow temperature range (3 K < T < 7 K). Remarkably, these oscillations can be understood in terms of magneto-phonon resonance originating from the interaction of 2DEG and leaky interface-acoustic phonon modes. The existence of such modes on the GaAs:AIGaAs interface is demonstrated theoretically and their velocities are calculated. It is shown that the electron-phonon scattering matrix element exhibits a peak for the phonons carrying momentum q = 2k{sub F} (k{sub F} is the Fermi wave-vector of 2DEG).
NASA Astrophysics Data System (ADS)
Liu, Houquan; Zhang, Xingchu
2017-03-01
In a semiconductor, optically excited electron-hole pairs, driven by a strong terahertz (THz) field, can recombine to create THz sidebands in the optical spectrum. The sideband spectrum exhibits a "plateau" up to a cutoff frequency of 3.17Up, where Up is the ponderomotive energy. In this letter, we predict that the bandwidth of this sideband spectrum plateau can be broadened by applying an additional direct-current (DC) electric field. We find that if applying a DC field of EDC=0.2ETHz (where EDC and ETHz are the amplitudes of the DC field and THz field, respectively), the sideband spectrum presents three plateaus with 5.8Up, 10.05Up and 16Up being the cutoff frequencies of the first, second and third plateaus, respectively. This bandwidth broadening occurs because the DC field can increase the kinetic energy that an electron-hole pair can gain from the THz field. This effect means that the bandwidth of the sideband spectrum can be controlled flexibly by changing the DC field, thereby facilitating the ultrafast electro-optical applications of THz sideband generation.
NASA Astrophysics Data System (ADS)
Sammut, L.; Messenger, C.; Melatos, A.; Owen, B. J.
2014-02-01
We describe the practical implementation of the sideband search, a search for periodic gravitational waves from neutron stars in binary systems. The orbital motion of the source in its binary system causes frequency modulation in the combination of matched filters known as the F-statistic. The sideband search is based on the incoherent summation of these frequency-modulated F-statistic sidebands. It provides a new detection statistic for sources in binary systems, called the C-statistic. The search is well suited to low-mass x-ray binaries, the brightest of which, called Sco X-1, is an ideal target candidate. For sources like Sco X-1, with well-constrained orbital parameters, a slight variation on the search is possible. The extra orbital information can be used to approximately demodulate the data from the binary orbital motion in the coherent stage, before incoherently summing the now reduced number of sidebands. We investigate this approach and show that it improves the sensitivity of the standard Sco X-1 directed sideband search. Prior information on the neutron star inclination and gravitational wave polarization can also be used to improve upper limit sensitivity. We estimate the sensitivity of a Sco X-1 directed sideband search on ten days of LIGO data and show that it can beat previous upper limits in current LIGO data, with a possibility of constraining theoretical upper limits using future advanced instruments.
Edge phonons in black phosphorus
Ribeiro, H. B.; Villegas, C. E. P.; Bahamon, D. A.; Muraca, D.; Castro Neto, A. H.; de Souza, E. A. T.; Rocha, A. R.; Pimenta, M. A.; de Matos, C. J. S.
2016-01-01
Black phosphorus has recently emerged as a new layered crystal that, due to its peculiar and anisotropic crystalline and electronic band structures, may have important applications in electronics, optoelectronics and photonics. Despite the fact that the edges of layered crystals host a range of singular properties whose characterization and exploitation are of utmost importance for device development, the edges of black phosphorus remain poorly characterized. In this work, the atomic structure and behaviour of phonons near different black phosphorus edges are experimentally and theoretically studied using Raman spectroscopy and density functional theory calculations. Polarized Raman results show the appearance of new modes at the edges of the sample, and their spectra depend on the atomic structure of the edges (zigzag or armchair). Theoretical simulations confirm that the new modes are due to edge phonon states that are forbidden in the bulk, and originated from the lattice termination rearrangements. PMID:27412813
Edge phonons in black phosphorus
NASA Astrophysics Data System (ADS)
Ribeiro, H. B.; Villegas, C. E. P.; Bahamon, D. A.; Muraca, D.; Castro Neto, A. H.; de Souza, E. A. T.; Rocha, A. R.; Pimenta, M. A.; de Matos, C. J. S.
2016-07-01
Black phosphorus has recently emerged as a new layered crystal that, due to its peculiar and anisotropic crystalline and electronic band structures, may have important applications in electronics, optoelectronics and photonics. Despite the fact that the edges of layered crystals host a range of singular properties whose characterization and exploitation are of utmost importance for device development, the edges of black phosphorus remain poorly characterized. In this work, the atomic structure and behaviour of phonons near different black phosphorus edges are experimentally and theoretically studied using Raman spectroscopy and density functional theory calculations. Polarized Raman results show the appearance of new modes at the edges of the sample, and their spectra depend on the atomic structure of the edges (zigzag or armchair). Theoretical simulations confirm that the new modes are due to edge phonon states that are forbidden in the bulk, and originated from the lattice termination rearrangements.
Hung, Ivan; Edwards, Trenton; Sen, Sabyasachi; Gan, Zhehong
2012-08-01
A Carr-Purcell Meiboom-Gill (CPMG) sensitivity-enhanced spinning sideband separation experiment is presented. The experiment combines the idea of magic-angle turning and phase-adjusted sideband separation (MATPASS), allowing for isotropic/anisotropic chemical shift separation of disordered solids with line widths far greater than the magic-angle spinning frequency. The use of CPMG enhances the sensitivity of the wide-line spectra by an order of magnitude via multiple-echo acquisition. The MATPASS/CPMG protocol involves acquisition of time-domain data using a MAT/CPMG pulse sequence followed by f(1) shearing during data processing to arrive at the PASS representation. Such a protocol has √2 higher sensitivity than the conventional PASS method because all CPMG echo signals are used for the final PASS spectrum. Application of this method is demonstrated using a GeSe₄ glass sample with both ⁷⁷Se isotropic line widths and chemical shift anisotropy that far exceed the spinning frequency. The sideband separation allows for the measurement of chemical shift anisotropy of the disordered solids.
NASA Astrophysics Data System (ADS)
Firla, Marcin; Li, Zhong-Yang; Martin, Nadine; Pachaud, Christian; Barszcz, Tomasz
2016-12-01
This paper proposes advanced signal-processing techniques to improve condition monitoring of operating machines. The proposed methods use the results of a blind spectrum interpretation that includes harmonic and sideband series detection. The first contribution of this study is an algorithm for automatic association of harmonic and sideband series to characteristic fault frequencies according to a kinematic configuration. The approach proposed has the advantage of taking into account a possible slip of the rolling-element bearings. In the second part, we propose a full-band demodulation process from all sidebands that are relevant to the spectral estimation. To do so, a multi-rate filtering process in an iterative schema provides satisfying precision and stability over the targeted demodulation band, even for unsymmetrical and extremely narrow bands. After synchronous averaging, the filtered signal is demodulated for calculation of the amplitude and frequency modulation functions, and then any features that indicate faults. Finally, the proposed algorithms are validated on vibration signals measured on a test rig that was designed as part of the European Innovation Project 'KAStrion'. This rig simulates a wind turbine drive train at a smaller scale. The data show the robustness of the method for localizing and extracting a fault on the main bearing. The evolution of the proposed features is a good indicator of the fault severity.
Generating controllable frequency-comb-like structures in terahertz range via Rabi sidebands
NASA Astrophysics Data System (ADS)
Filin, Alex; Romanov, Dmitri; Levis, Robert
2013-05-01
When broad, coherent Rabi sidebands are invoked by a moderately intense picosecond laser pulse, they typically exhibit spectral interference fringes. We demonstrate the possibility of controlling this fringe pattern toward a comb-like structure. We investigated the influence of the driving pulse (normalized to 1 ps FWHM) shape parameters on the structural characteristics of the sideband spectra: the spectrum envelope, the fringe contrast, and the fringe spacing variation. The envelope was found to depend drastically on the sharpness of the driving pulse, that is, on the rate at which the temporal distance between the leading and trailing edges grows away from the pulse maximum. Increase in this parameter effectively flattens the envelope. The fringe contrast, that is, the maximum-to-minimum difference, depends strongly on the asymmetry of the driving pulse. The imbalance between the driving and the trailing edges leads to fast decrease of the contrast. The variation of inter-peak distance within a sideband was controlled using super-Gaussian shape of the driving pulse. While for the Gaussian pulse the inter-peak distance increases almost 5 times over the interval from 1.60 to 1.66 eV (in the case of oxygen), sufficiently super-Gaussian shape leads to almost equidistant fringes (comb-like spectrum). Support from the Air Force Office of Scientific Research, Grant No. N00014-10-0293, is gratefully acknowledged.
Yan, Zhequan; Chen, Liang; Yoon, Mina; Kumar, Satish
2016-02-21
Hexagonal boron nitride (h-BN) is a promising substrate for graphene based nano-electronic devices. We investigate the ballistic phonon transport at the interface of vertically stacked graphene and h-BN heterostructures using first principles density functional theory and atomistic Green's function simulations considering the influence of lattice stacking. We compute the frequency and wave-vector dependent transmission function and observe distinct stacking-dependent phonon transmission features for the h-BN/graphene/h-BN sandwiched systems. We find that the in-plane acoustic modes have the dominant contributions to the phonon transmission and thermal boundary conductance (TBC) for the interfaces with the carbon atom located directly on top of the boron atom (C-B matched) because of low interfacial spacing. The low interfacial spacing is a consequence of the differences in the effective atomic volume of N and B and the difference in the local electron density around N and B. For the structures with the carbon atom directly on top of the nitrogen atom (C-N matched), the spatial distance increases and the contribution of in-plane modes to the TBC decreases leading to higher contributions by out-of-plane acoustic modes. We find that the C-B matched interfaces have stronger phonon-phonon coupling than the C-N matched interfaces, which results in significantly higher TBC (more than 50%) in the C-B matched interface. The findings in this study will provide insights to understand the mechanism of phonon transport at h-BN/graphene/h-BN interfaces, to better explain the experimental observations and to engineer these interfaces to enhance heat dissipation in graphene based electronic devices.
NASA Astrophysics Data System (ADS)
Yan, Zhequan; Chen, Liang; Yoon, Mina; Kumar, Satish
2016-02-01
Hexagonal boron nitride (h-BN) is a promising substrate for graphene based nano-electronic devices. We investigate the ballistic phonon transport at the interface of vertically stacked graphene and h-BN heterostructures using first principles density functional theory and atomistic Green's function simulations considering the influence of lattice stacking. We compute the frequency and wave-vector dependent transmission function and observe distinct stacking-dependent phonon transmission features for the h-BN/graphene/h-BN sandwiched systems. We find that the in-plane acoustic modes have the dominant contributions to the phonon transmission and thermal boundary conductance (TBC) for the interfaces with the carbon atom located directly on top of the boron atom (C-B matched) because of low interfacial spacing. The low interfacial spacing is a consequence of the differences in the effective atomic volume of N and B and the difference in the local electron density around N and B. For the structures with the carbon atom directly on top of the nitrogen atom (C-N matched), the spatial distance increases and the contribution of in-plane modes to the TBC decreases leading to higher contributions by out-of-plane acoustic modes. We find that the C-B matched interfaces have stronger phonon-phonon coupling than the C-N matched interfaces, which results in significantly higher TBC (more than 50%) in the C-B matched interface. The findings in this study will provide insights to understand the mechanism of phonon transport at h-BN/graphene/h-BN interfaces, to better explain the experimental observations and to engineer these interfaces to enhance heat dissipation in graphene based electronic devices.
Measuring phonons in protein crystals
NASA Astrophysics Data System (ADS)
Niessen, Katherine A.; Snell, Edward; Markelz, A. G.
2013-03-01
Using Terahertz near field microscopy we find orientation dependent narrow band absorption features for lysozyme crystals. Here we discuss identification of protein collective modes associated with the observed features. Using normal mode calculations we find good agreement with several of the measured features, suggesting that the modes arise from internal molecular motions and not crystal phonons. Such internal modes have been associated with protein function.
Prospective Solid-state Photonic Cryocooler Based on the "Phonon-deficit Effect"
NASA Astrophysics Data System (ADS)
Melkonyan, Gurgen; Gulian, Armen
In this design microwave photons are propagating in a sapphire rod, and are being absorbed by a superconductor deposited on the surface of the rod. The frequency of the radiation is tuned to be less than the energy gap in the superconductor, so that the pair breaking is not taking place. This photon pumping redistributes the electron-hole quasiparticles: their distribution function is non-equilibrium, and the "phonon-deficit effect" takes place. There is a dielectric material deposited on top of superconductor, which serves asthe "cold finger" of the cooler. Its "acoustical density" is supposed to be smaller than that of the superconducting material, so phonons are being "rectified" and propagate from, but not to it: the energy flows from the "cold finger" into the superconductor. The best reported rectification achieved as of today is about factor of five, which is marginal for our design. To further enhance the rectification, one can use the acoustical filtering. It can be arranged between the superconductor and the "cold finger". Having a remarkably high heat conductivity and high acoustic density, the sapphire rod serves not only as a photonic wave-guide, but also as a thermal heat sink. It is thermally anchored to the bigger external heat-bath. Spectral phonon filters are arranged between sapphire and superconducting film, so that sapphire would only receive and absorb excess phonons without supplying deficient phonons to the superconductor. We performed calculations using parameters of existing materials;majordetails characterizing the designhave been taken into account. Opportunities are "cool" enough to be pursued experimentally.
NASA Astrophysics Data System (ADS)
Tsai, Chia-Nien; Chen, Lien-Wen
2016-07-01
Self-collimation is wave propagation in straight path without diffraction. The performance is evaluated by bandwidth, angular collimating range and straightness of equi-frequency contours. The present study aims to manipulate the self-collimated beam in square-array phononic crystals by means of orientated rectangular inclusions. Finite element simulations are performed to investigate the effects of the aspect ratio and orientation angle of rectangular inclusions on the self-collimated beam. The simulation results show that the proposed design successfully achieves all-angle self-collimation phenomenon. In addition, it also shows that the propagation direction of a self-collimated beam can be effectively manipulated by varying the orientation angle of inclusions. Numerical simulation result of the S-shaped bend demonstrates that acoustic collimated beam can be steered with negligible diffraction. Overall, the proposed design has significant potential for the realization of applications such as collimators, acoustic waveguides and other phononic crystals-based systems.
NASA Astrophysics Data System (ADS)
Ma, Hao; Li, Chen; Tang, Shixiong; Yan, Jiaqiang; Alatas, Ahmet; Lindsay, Lucas; Sales, Brian C.; Tian, Zhiting
2016-12-01
Cubic boron arsenide (BAs) was predicted to have an exceptionally high thermal conductivity (k ) ˜2000 W m-1K-1 at room temperature, comparable to that of diamond, based on first-principles calculations. Subsequent experimental measurements, however, only obtained a k of ˜200 W m-1K-1 . To gain insight into this discrepancy, we measured phonon dispersion of single-crystal BAs along high symmetry directions using inelastic x-ray scattering and compared these with first-principles calculations. Based on the measured phonon dispersion, we have validated the theoretical prediction of a large frequency gap between acoustic and optical modes and bunching of acoustic branches, which were considered the main reasons for the predicted ultrahigh k . This supports its potential to be a super thermal conductor if very-high-quality single-crystal samples can be synthesized.
Ma, Hao; Li, Chen; Tang, Shixiong; ...
2016-12-14
Cubic boron arsenide (BAs) was predicted to have an exceptionally high thermal conductivity (k) ~2000 Wm-1K-1 at room temperature, comparable to that of diamond, based on first-principles calculations. Subsequent experimental measurements, however, only obtained a k of ~200 Wm-1K-1. To gain insight into this discrepancy, we measured phonon dispersion of single crystal BAs along high symmetry directions using inelastic x-ray scattering (IXS) and compared these with first-principles calculations. Based on the measured phonon dispersion, we have validated the theoretical prediction of a large frequency gap between acoustic and optical modes and bunching of acoustic branches, which were considered the mainmore » reasons for the predicted ultrahigh k. This supports its potential to be a super thermal conductor if very high-quality single crystal samples can be synthesized.« less
NASA Astrophysics Data System (ADS)
Madrid, Angeline; Kim, Hyeon-Deuk; Habenicht, Bradley; Prezhdo, Oleg
2010-03-01
Phonon-induced dephasing processes that govern optical line widths, multiple exciton (ME) generation (MEG), and ME fission (MEF) in semiconductor quantum dots (QDs) are investigated by ab initio molecular dynamics simulation. Using Si QDs as an example, we propose that MEF occurs by phonon-induced dephasing and, for the first time, estimate its time scale to be 100 fs. In contrast, luminescence and MEG dephasing times are all sub-10 fs. Generally, dephasing is faster for higher-energy and higher-order excitons and increased temperatures. MEF is slow because it is facilitated only by low-frequency acoustic modes. Luminescence and MEG couple to both acoustic and optical modes of the QD, as well as ligand vibrations. The detailed atomistic simulation of the dephasing processes advances understanding of exciton dynamics in QDs and other nanoscale materials.
Ma, Hao; Li, Chen; Tang, Shixiong; Yan, Jiaqiang; Alatas, Ahmet; Lindsay, Lucas; Sales, Brian C.; Tian, Zhiting
2016-12-14
Cubic boron arsenide (BAs) was predicted to have an exceptionally high thermal conductivity (k) ~2000 Wm^{-1}K^{-1} at room temperature, comparable to that of diamond, based on first-principles calculations. Subsequent experimental measurements, however, only obtained a k of ~200 Wm-1K-1. To gain insight into this discrepancy, we measured phonon dispersion of single crystal BAs along high symmetry directions using inelastic x-ray scattering (IXS) and compared these with first-principles calculations. Based on the measured phonon dispersion, we have validated the theoretical prediction of a large frequency gap between acoustic and optical modes and bunching of acoustic branches, which were considered the main reasons for the predicted ultrahigh k. This supports its potential to be a super thermal conductor if very high-quality single crystal samples can be synthesized.
NASA Astrophysics Data System (ADS)
Agyare, Benjamin; Riseborough, Peter
2017-01-01
Intrinsically Localized Modes (ILMs) have purportedly been observed in NaI but only for wave-vectors, q at the corner of the 3-D Brillouin Zone. It has been suggested that, for high-symmetry q vectors, several van Hove singularities may converge at one frequency producing a large peak in the two-phonon density of state and giving rise to ILMs with these q values. We fit the experimentally determined acoustic and the optic phonon modes using a nearest neighbor and a next-nearest neighbor force constant. We find that the two-phonon density of states, for fixed q exhibits non-divergent van Hove singularities. The frequencies of these features are found to vary as q is varied. We intend to search for q values at which the two-phonon density of states is enhanced and then examine whether the anharmonic interactions can bind the two-phonon excitations to produce a quantized ILM.
Scanning Tunneling Microscopy Observation of Phonon Condensate.
Altfeder, Igor; Voevodin, Andrey A; Check, Michael H; Eichfeld, Sarah M; Robinson, Joshua A; Balatsky, Alexander V
2017-02-22
Using quantum tunneling of electrons into vibrating surface atoms, phonon oscillations can be observed on the atomic scale. Phonon interference patterns with unusually large signal amplitudes have been revealed by scanning tunneling microscopy in intercalated van der Waals heterostructures. Our results show that the effective radius of these phonon quasi-bound states, the real-space distribution of phonon standing wave amplitudes, the scattering phase shifts, and the nonlinear intermode coupling strongly depend on the presence of defect-induced scattering resonance. The observed coherence of these quasi-bound states most likely arises from phase- and frequency-synchronized dynamics of all phonon modes, and indicates the formation of many-body condensate of optical phonons around resonant defects. We found that increasing the strength of the scattering resonance causes the increase of the condensate droplet radius without affecting the condensate fraction inside it. The condensate can be observed at room temperature.
Scanning Tunneling Microscopy Observation of Phonon Condensate
Altfeder, Igor; Voevodin, Andrey A.; Check, Michael H.; Eichfeld, Sarah M.; Robinson, Joshua A.; Balatsky, Alexander V.
2017-01-01
Using quantum tunneling of electrons into vibrating surface atoms, phonon oscillations can be observed on the atomic scale. Phonon interference patterns with unusually large signal amplitudes have been revealed by scanning tunneling microscopy in intercalated van der Waals heterostructures. Our results show that the effective radius of these phonon quasi-bound states, the real-space distribution of phonon standing wave amplitudes, the scattering phase shifts, and the nonlinear intermode coupling strongly depend on the presence of defect-induced scattering resonance. The observed coherence of these quasi-bound states most likely arises from phase- and frequency-synchronized dynamics of all phonon modes, and indicates the formation of many-body condensate of optical phonons around resonant defects. We found that increasing the strength of the scattering resonance causes the increase of the condensate droplet radius without affecting the condensate fraction inside it. The condensate can be observed at room temperature. PMID:28225066
Scanning phononic lattices with ultrasound
Vines, R.E.; Wolfe, J.P.; Every, A.V.
1999-11-01
A method for probing the elastic properties of newly developed periodic structures using acoustic waves is introduced. Highly anisotropic transmission of surface acoustic waves is observed by continuously scanning the wave vector angle. Preliminary models of wave propagation through multilayers and two-dimensional lattices explain some of the experimental features, while other features can be attributed to the resonant excitation of interface waves. {copyright} {ital 1999} {ital The American Physical Society}
An acoustic neuroma is a benign tumor that develops on the nerve that connects the ear to the brain. ... can press against the brain, becoming life-threatening. Acoustic neuroma can be difficult to diagnose, because the ...
Coherent Phonon Rabi Oscillations with a High-Frequency Carbon Nanotube Phonon Cavity.
Zhu, Dong; Wang, Xin-He; Kong, Wei-Cheng; Deng, Guang-Wei; Wang, Jiang-Tao; Li, Hai-Ou; Cao, Gang; Xiao, Ming; Jiang, Kai-Li; Dai, Xing-Can; Guo, Guang-Can; Nori, Franco; Guo, Guo-Ping
2017-02-08
Phonon-cavity electromechanics allows the manipulation of mechanical oscillations similar to photon-cavity systems. Many advances on this subject have been achieved in various materials. In addition, the coherent phonon transfer (phonon Rabi oscillations) between the phonon cavity mode and another oscillation mode has attracted many interest in nanoscience. Here, we demonstrate coherent phonon transfer in a carbon nanotube phonon-cavity system with two mechanical modes exhibiting strong dynamical coupling. The gate-tunable phonon oscillation modes are manipulated and detected by extending the red-detuned pump idea of photonic cavity electromechanics. The first- and second-order coherent phonon transfers are observed with Rabi frequencies 591 and 125 kHz, respectively. The frequency quality factor product fQm ∼ 2 × 10(12) Hz achieved here is larger than kBTbase/h, which may enable the future realization of Rabi oscillations in the quantum regime.
Extraordinary lateral beaming of sound from a square-lattice phononic crystal
NASA Astrophysics Data System (ADS)
Bai, Xiaoxue; Qiu, Chunyin; He, Hailong; Peng, Shasha; Ke, Manzhu; Liu, Zhengyou
2017-03-01
This work revisits the sound transmission through a finite phononic crystal of square lattice. In addition to a direct, ordinary transmission through the sample, an extraordinary lateral beaming effect is also observed. The phenomenon stems from the equivalence of the states located around the four corners of the first Brillouin zone. The experimental result agrees well with the theoretical prediction. The lateral beaming behavior enables a simple design for realizing acoustic beam splitters.
On-chip optical mode conversion based on dynamic grating in photonic-phononic hybrid waveguide
Chen, Guodong; Zhang, Ruiwen; Sun, Junqiang
2015-01-01
We present a scheme for reversible and tunable on-chip optical mode conversion based on dynamic grating in a hybrid photonic-phononic waveguide. The dynamic grating is built up through the acousto-optic effect and the theoretical model of the optical mode conversion is developed by considering the geometrical deformation and refractive index change. Three kinds of mode conversions are able to be realized using the same hybrid waveguide structure in a large bandwidth by only changing the launched acoustic frequency. The complete mode conversion can be achieved by choosing a proper acoustic power under a given waveguide length. PMID:25996236
Strong coupling between phonons and optical beating in backward Brillouin scattering
NASA Astrophysics Data System (ADS)
Huy, Kien Phan; Beugnot, Jean-Charles; Tchahame, Joël-Cabrel; Sylvestre, Thibaut
2016-10-01
Brillouin scattering is a fundamental nonlinear interaction between two optical waves and an acoustic wave mediated by electrostriction and photoelasticity. In this paper, we revisit the usual theory of this inelastic scattering to get a joint system in which the acoustic wave is strongly coupled to the interference pattern between the optical waves. We show in particular that when the coupling rate exceeds the phonon damping rate, the system enters the strong-coupling regime, giving rise to anticrossing in the dispersion relation and Rabi-like splitting. We further find numerically that strong coupling can, in principle, be observed using backward Brillouin scattering in subwavelength-diameter optical waveguides.
Temperature Dependence of Phonons in Pyrolitic Graphite
DOE R&D Accomplishments Database
Brockhouse, B. N.; Shirane, G.
1977-01-01
Dispersion curves for longitudinal and transverse phonons propagating along and near the c-axis in pyrolitic graphite at temperatures between 4°K and 1500°C have been measured by neutron spectroscopy. The observed frequencies decrease markedly with increasing temperature (except for the transverse optical ''rippling'' modes in the hexagonal planes). The neutron groups show interesting asymmetrical broadening ascribed to interference between one phonon and many phonon processes.
Phonon-induced diamagnetic force and its effect on the lattice thermal conductivity.
Jin, Hyungyu; Restrepo, Oscar D; Antolin, Nikolas; Boona, Stephen R; Windl, Wolfgang; Myers, Roberto C; Heremans, Joseph P
2015-06-01
Phonons are displacements of atoms around their rest positions in a crystalline solid. They carry sound and heat, but are not classically associated with magnetism. Here, we show that phonons are, in fact, sensitive to magnetic fields, even in diamagnetic materials. We do so by demonstrating experimentally that acoustic phonons in a diamagnetic semiconductor (InSb) scatter more strongly from one another when a magnetic field is applied. We attribute this observation to the magnetic-field sensitivity of the anharmonicity of the interatomic bonds that govern the probability of phonon-phonon interactions. The displacements of atoms locally affect the orbital motion of valence band electrons, which, in the presence of an external magnetic field, spatially modulates the orbital diamagnetism around the displaced atoms. The spatial gradient in magnetic moment results in an anharmonic magnetic force exerted on the displaced atom. The process is modelled by ab initio calculations that, without the use of a single adjustable parameter, reproduce the observed 12% decrease in the lattice thermal conductivity under a 7 T magnetic field at a temperature of 5.2 K.
Influence of phonon reservoir on photon blockade in a driven quantum dot-cavity system
NASA Astrophysics Data System (ADS)
Gao, Bo; Zhu, Jia-pei; Li, Gao-xiang
2016-03-01
We theoretically investigate the influence of the phonon bath on photon blockade in a simultaneously driven dot-cavity system. An optimal condition for avoiding two-photon excitation of a cavity field is put forward which can be achieved by modulating the phase difference and the strengths of the driving fields. The second-order correlation function and the mean photon number of the cavity field are discussed. In the absence of phonon effect, the strong photon blockade in a moderate quantum dot (QD)-cavity coupling regime occurs, which can be attributed to the destructive quantum interference arisen from different transition paths induced by simultaneously driving the dressed QD-cavity system. The participation of acoustic-phonon reservoir produces new transition channels for the QD-cavity system, which leads to the damage of destructive interference. As a result, the photon blockade effect is hindered when taking the electron-phonon interaction into account. It is also found that the temperature of the phonon reservoir is disadvantageous for the generation of photon blockade.
2008-03-07
a national naval responsibility. Acoustic sensors on mobile, autonomous platforms will enable basic research topics on temporal and spatial...problem and acoustic navigation and communications within the context of distributed autonomous persistent undersea surveillance sensor networks...Acoustic sensors on mobile, autonomous platforms will enable basic research topics on temporal and spatial coherence and the description of ambient
NASA Technical Reports Server (NTRS)
Steinetz, Bruce M. (Inventor)
2006-01-01
The invention relates to a sealing device having an acoustic resonator. The acoustic resonator is adapted to create acoustic waveforms to generate a sealing pressure barrier blocking fluid flow from a high pressure area to a lower pressure area. The sealing device permits noncontacting sealing operation. The sealing device may include a resonant-macrosonic-synthesis (RMS) resonator.
NASA Technical Reports Server (NTRS)
Steinetz, Bruce M. (Inventor)
2006-01-01
The invention relates to a sealing device having an acoustic resonator. The acoustic resonator is adapted to create acoustic waveforms to generate a sealing pressure barrier blocking fluid flow from a high pressure area to a lower pressure area. The sealing device permits noncontacting sealing operation. The sealing device may include a resonant-macrosonic-synthesis (RMS) resonator.
Electron-phonon interactions from first principles
NASA Astrophysics Data System (ADS)
Giustino, Feliciano
2017-01-01
This article reviews the theory of electron-phonon interactions in solids from the point of view of ab initio calculations. While the electron-phonon interaction has been studied for almost a century, predictive nonempirical calculations have become feasible only during the past two decades. Today it is possible to calculate from first principles many materials properties related to the electron-phonon interaction, including the critical temperature of conventional superconductors, the carrier mobility in semiconductors, the temperature dependence of optical spectra in direct and indirect-gap semiconductors, the relaxation rates of photoexcited carriers, the electron mass renormalization in angle-resolved photoelectron spectra, and the nonadiabatic corrections to phonon dispersion relations. In this article a review of the theoretical and computational framework underlying modern electron-phonon calculations from first principles as well as landmark investigations of the electron-phonon interaction in real materials is given. The first part of the article summarizes the elementary theory of electron-phonon interactions and their calculations based on density-functional theory. The second part discusses a general field-theoretic formulation of the electron-phonon problem and establishes the connection with practical first-principles calculations. The third part reviews a number of recent investigations of electron-phonon interactions in the areas of vibrational spectroscopy, photoelectron spectroscopy, optical spectroscopy, transport, and superconductivity.
Phonon-assisted transient electroluminescence in Si
Cheng, Tzu-Huan; Chu-Su, Yu; Liu, Chien-Sheng; Lin, Chii-Wann
2014-06-30
The phonon-replica infrared emission is observed at room temperature from indirect band gap Si light-emitting diode under forward bias. With increasing injection current density, the broadened electroluminescence spectrum and band gap reduction are observed due to joule heating. The spectral-resolved temporal response of electroluminescence reveals the competitiveness between single (TO) and dual (TO + TA) phonon-assisted indirect band gap transitions. As compared to infrared emission with TO phonon-replica, the retarder of radiative recombination at long wavelength region (∼1.2 μm) indicates lower transition probability of dual phonon-replica before thermal equivalent.
Effect of Rattling Phonons on Sommerfeld Constant
NASA Astrophysics Data System (ADS)
Hotta, Takashi
2008-10-01
By employing a numerical renormalization group technique, we evaluate electronic specific heat coefficient γ of the Anderson model coupled with local anharmonic phonons for the oscillation of a caged atom. For the rattling-type cage potential with a flat and wide region in the bottom, we find that phonon-mediated attraction is largely enhanced. When the potential shape is deformed from the rattling type, there occurs a cancellation between Coulomb repulsion and the phonon-mediated attraction. In such a situation, spin and charge fluctuations are comparable to each other, leading to the realization of exotic electron-phonon complex state with large and magnetically robust γ.
Band structures in two-dimensional phononic crystals with periodic Jerusalem cross slot
NASA Astrophysics Data System (ADS)
Li, Yinggang; Chen, Tianning; Wang, Xiaopeng; Yu, Kunpeng; Song, Ruifang
2015-01-01
In this paper, a novel two-dimensional phononic crystal composed of periodic Jerusalem cross slot in air matrix with a square lattice is presented. The dispersion relations and the transmission coefficient spectra are calculated by using the finite element method based on the Bloch theorem. The formation mechanisms of the band gaps are analyzed based on the acoustic mode analysis. Numerical results show that the proposed phononic crystal structure can yield large band gaps in the low-frequency range. The formation mechanism of opening the acoustic band gaps is mainly attributed to the resonance modes of the cavities inside the Jerusalem cross slot structure. Furthermore, the effects of the geometrical parameters on the band gaps are further explored numerically. Results show that the band gaps can be modulated in an extremely large frequency range by the geometry parameters such as the slot length and width. These properties of acoustic waves in the proposed phononic crystals can potentially be applied to optimize band gaps and generate low-frequency filters and waveguides.
Non-equilibrium optical phonon dynamics in bulk and low-dimensional semiconductors
NASA Astrophysics Data System (ADS)
Srivastava, G. P.
2007-02-01
We present theoretical investigations of the intrinsic dynamics of long-wavelength non-equilibrium optical phonons in bulk and low-dimensional semiconductors. The theory is based on the application of Fermi's golden rule formula, with phonon dispersion relations as well as crystal anharmonicity considered in the framework of isotropic continuum model. Contributions to the decay rates of the phonon modes are discussed in terms of four possible channels: Klemens channel (into two acoustic daughter modes), generalised Ridley channel (into one acoustic and one optical mode), generalised Vallee-Bogani channel (into a lower mode of the same branch and an acoustic mode), and Barman-Srivastava channel (into two lower-branch optical modes). The role of crystal structure and cation/anion mass ratio in determining the lifetime of such modes in bulk semiconductors is highlighted. Estimates of lifetimes of such modes in silicon nanowires and carbon nanotubes will also be presented. The results support and explain available experimental data, and make predictions in some cases.
Thin Superconducting Film Characterization by Surface Acoustic Waves.
2014-09-26
NUMBER 2. GOVT ACCESSION NO. 3 RECIPIENT’S CA ALOG NUMBER ~~AFOSR TR -0 8 4. TITLE (and Subtitle) 5 TYPE OF REPORT & PERIOD COVERED Thin Superconducting ...thin film superconductor surface acoustic waves I SAW electron phonon interaction superconducting energy gap electron mean free path vortex...electrical resistivity and the attenuation of surface ,e J -acoustic waves (SAW) were measured in the superconducting state of a L granular lead film
Nonlinear ultrafast acoustics at the nano scale.
van Capel, P J S; Péronne, E; Dijkhuis, J I
2015-02-01
Pulsed femtosecond lasers can generate acoustic pulses propagating in solids while displaying either diffraction, attenuation, nonlinearity and/or dispersion. When acoustic attenuation and diffraction are negligible, shock waves or solitons can form during propagation. Both wave types are phonon wavepackets with characteristic length scales as short as a few nanometer. Hence, they are well suited for acoustic characterization and manipulation of materials on both ultrafast and ultrashort scales. This work presents an overview of nonlinear ultrasonics since its first experimental demonstration at the beginning of this century to the more recent developments. We start by reviewing the main properties of nonlinear ultrafast acoustic propagation based on the underlying equations. Then we show various results obtained by different groups around the world with an emphasis on recent work. Current issues and directions of future research are discussed.
Mante, Pierre-Adrien; Chen, Chien-Cheng; Wen, Yu-Chieh; Sheu, Jinn-Kong; Sun, Chi-Kuang
2013-11-27
A phonon nanoscopy method, based on the picosecond ultrasonics technique, capable of studying the complex acoustic reflection coefficient at frequency up to 1 THz is proposed and demonstrated. By measuring the reflection coefficient at the same surface location at the interface between GaN and air, and between GaN and the material to characterize, we get access to the THz amplitude and phase spectra of the acoustic phonon reflection. The retrieval of both these pieces of information then allows the calculation of the attenuation in a wide range of frequency and gives new insight into the Kapitza anomaly. This method is then applied to cubic ice, and the measurements of the elastic properties, the phonon anharmonic decay spectrum up to 1 THz, as well as the measurements of the thermal phonon lifetime at 150 K are all achieved.
Scattering Tools for Nanostructure Phonon Engineering
2013-09-25
Arlington, VA 22203 AFOSR The vibrational properties of solids have crucial roles underpinning functional properties ranging from thermal conductivity... thermal diffuse scattering (TDS) techniques to nanoscale systems. With this approach we can probe phonons across the nanomaterials, phonons, x-ray...scattering, nanomembrane fabrication, flatness, large-wavevector vibrational properties, synchrotron x-rays, thermal diffuse scattering, silicon
Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe1-xMxSi (M =Ir , Os )
NASA Astrophysics Data System (ADS)
Delaire, O.; Al-Qasir, I. I.; May, A. F.; Li, C. W.; Sales, B. C.; Niedziela, J. L.; Ma, J.; Matsuda, M.; Abernathy, D. L.; Berlijn, T.
2015-03-01
The vibrational behavior of heavy substitutional impurities (M = Ir,Os) in Fe1-xMxSi (x =0 ,0.02 ,0.04 ,0.1 ) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. Our INS measurements on single crystals mapped the four-dimensional dynamical structure factor, S (Q ,E ) , for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers, leads to softened interatomic force constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S (Q ,E ) from INS through a Green's-function model incorporating the phonon self-energy based on first-principles density functional theory simulations, and we study the disorder-induced lifetimes on large supercells. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.
An optically controlled phased array antenna based on single sideband polarization modulation.
Zhang, Yamei; Wu, Huan; Zhu, Dan; Pan, Shilong
2014-02-24
A novel optically controlled phased array antenna consisting a simple optical beamforming network and an N element linear patch antenna array is proposed and demonstrated. The optical beamforming network is realized by N independent phase shifters using a shared optical single sideband (OSSB) polarization modulator together with N polarization controllers (PCs), N polarization beam splitters (PBSs) and N photodetectors (PDs). An experiment is carried out. A 4-element linear patch antenna array operating at 14 GHz and a 1 × 4 optical beamforming network (OBFN) is employed to realize the phased array antenna. The radiation patterns of the phased array antenna at -30°, 0° and 30° are achieved.
Configuration-constrained cranking Hartree-Fock pairing calculations for sidebands of nuclei
NASA Astrophysics Data System (ADS)
Liang, W. Y.; Jiao, C. F.; Wu, Q.; Fu, X. M.; Xu, F. R.
2015-12-01
Background: Nuclear collective rotations have been successfully described by the cranking Hartree-Fock-Bogoliubov (HFB) model. However, for rotational sidebands which are built on intrinsic excited configurations, it may not be easy to find converged cranking HFB solutions. The nonconservation of the particle number in the BCS pairing is another shortcoming. To improve the pairing treatment, a particle-number-conserving (PNC) pairing method was suggested. But the existing PNC calculations were performed within a phenomenological one-body potential (e.g., Nilsson or Woods-Saxon) in which one has to deal the double-counting problem. Purpose: The present work aims at an improved description of nuclear rotations, particularly for the rotations of excited configurations, i.e., sidebands. Methods: We developed a configuration-constrained cranking Skyrme Hartree-Fock (SHF) calculation with the pairing correlation treated by the PNC method. The PNC pairing takes the philosophy of the shell model which diagonalizes the Hamiltonian in a truncated model space. The cranked deformed SHF basis provides a small but efficient model space for the PNC diagonalization. Results: We have applied the present method to the calculations of collective rotations of hafnium isotopes for both ground-state bands and sidebands, reproducing well experimental observations. The first up-bendings observed in the yrast bands of the hafnium isotopes are reproduced, and the second up-bendings are predicted. Calculations for rotational bands built on broken-pair excited configurations agree well with experimental data. The band-mixing between two Kπ=6+ bands observed in 176Hf and the K purity of the 178Hf rotational state built on the famous 31 yr Kπ=16+ isomer are discussed. Conclusions: The developed configuration-constrained cranking calculation has been proved to be a powerful tool to describe both the yrast bands and sidebands of deformed nuclei. The analyses of rotational moments of inertia
Giant-laser-pulse-induced Rabi sideband of a multilevel dressed atom
NASA Astrophysics Data System (ADS)
Chen, Tian-Jie; Duan, Shao-Guang
1993-03-01
Rabi sidebands of the Na atomic vapor excited by a resonant-pulsed-laser beam were observed in the forward-direction radiation. While the laser power scans over a factor of 10, the change of Rabi shift is much less than what is expected by the two-level dressed-atom model. Therefore a multilevel dressed-atom model is developed to calculate the levels of the dressed Na atom, and the influence of the time evolution of the laser power is also taken into account in counting the real observable spectrum. After considering all these factors, the final calculated data fit the experimental results satisfactorily.
NASA Astrophysics Data System (ADS)
Ju, Cheng; Chen, Xue; Liu, Na; Wang, Liqian
2014-09-01
The presence of vestigial-sideband optical filter, dispersion and chirp of modulator increases subcarrier to subcarrier intermixing interference (SSII), which significantly restricts transmission performance. For the first time, the iterative interference cancellation method is introduced to calculate and eliminate SSII. Furthermore, we successfully demonstrate a 40-Gbps, 16-QAM, dual drive Mach-Zehnder modulator (MZM)-based system transmission through 100-km uncompensated standard single-mode fiber. The impact of chirp on iterative algorithm is also experimentally evaluated by setting different optical phase modulation amplitudes on the two arms of the dual drive MZM.
Hangauer, Andreas; Spinner, Georg; Nikodem, Michal; Wysocki, Gerard
2014-09-22
Both intensity- (IM) and frequency-modulation (FM) behavior of a directly modulated quantum cascade laser (QCL) are measured from 300 Hz to 1.7 GHz. Quantitative measurements of tuning coefficients has been performed and the transition from thermal- to electronic-tuning is clearly observed. A very specific FM behavior of QCLs has been identified which allows for optical quasi single sideband (SSB) modulation through current injection and has not been observed in directly modulated semiconductor lasers before. This predestines QCLs in applications where SSB is required, such as telecommunication or high speed spectroscopy. The experimental procedure and theoretical modeling for data extraction is discussed.
Parametric instabilities of large amplitude Alfven waves with obliquely propagating sidebands
NASA Technical Reports Server (NTRS)
Vinas, A. F.; Goldstein, M. L.
1992-01-01
This paper presents a brief report on properties of the parametric decay and modulational, filamentation, and magnetoacoustic instabilities of a large amplitude, circularly polarized Alfven wave. We allow the daughter and sideband waves to propagate at an arbitrary angle to the background magnetic field so that the electrostatic and electromagnetic characteristics of these waves are coupled. We investigate the dependance of these instabilities on dispersion, plasma/beta, pump wave amplitude, and propagation angle. Analytical and numerical results are compared with numerical simulations to investigate the full nonlinear evolution of these instabilities.
Unexpected non-local effects in dual-probe-sideband BOTDA
NASA Astrophysics Data System (ADS)
Dominguez-Lopez, Alejandro; Angulo-Vinuesa, Xabier; Lopez-Gil, Alexia; Martin-Lopez, Sonia; Gonzalez-Herraez, Miguel
2015-09-01
Until now, non-local effects in dual-probe-sideband Brillouin Optical Time Domain Analysis (BOTDA) systems have been considered negligible if the probe power is below the Stimulated Brillouin Scattering (SBS) threshold. In this paper, we show the appearance of non-local effects even below the SBS threshold. The pump pulse experiences a frequency dependent spectral deformation that affects the readout process differently in the gain and loss configurations. The main conclusion of our study is that the measurements in gain configuration are more robust to this non-local effect than the loss configuration. These results are of particular interest for manufacturers of long-range BOTDA systems.
NASA Technical Reports Server (NTRS)
Farhoomand, J.; Pickett, H. M.; Blake, G. A.
1985-01-01
The direct (zero-field) spectra of the fundamental rotational transitions of the OH radical in its Omega = 3/2 and 1/2 states at 2509.9 and 1834.7 GHz are obtained using a recently developed far-infrared laser sideband spectrometer. These measurements have verified and refined the predictions of previous laser magnetic resonance work, thereby confirming the far-infrared detection of interstellar OH. The increased accuracy of these direct measurements will be useful to future astronomical and atmospheric studies of these important transitions.
Lattice Boltzmann modeling of phonon transport
NASA Astrophysics Data System (ADS)
Guo, Yangyu; Wang, Moran
2016-06-01
A novel lattice Boltzmann scheme is proposed for phonon transport based on the phonon Boltzmann equation. Through the Chapman-Enskog expansion, the phonon lattice Boltzmann equation under the gray relaxation time approximation recovers the classical Fourier's law in the diffusive limit. The numerical parameters in the lattice Boltzmann model are therefore rigorously correlated to the bulk material properties. The new scheme does not only eliminate the fictitious phonon speed in the diagonal direction of a square lattice system in the previous lattice Boltzmann models, but also displays very robust performances in predicting both temperature and heat flux distributions consistent with analytical solutions for diverse numerical cases, including steady-state and transient, macroscale and microscale, one-dimensional and multi-dimensional phonon heat transport. This method may provide a powerful numerical tool for deep studies of nonlinear and nonlocal heat transports in nanosystems.
Ultrafast Structure Switching through Nonlinear Phononics
NASA Astrophysics Data System (ADS)
Juraschek, D. M.; Fechner, M.; Spaldin, N. A.
2017-02-01
We describe a mechanism by which nonlinear phononics allows ultrafast coherent and directional control of transient structural distortions. With ErFeO3 as a model system, we use density functional theory to calculate the structural properties as input into an anharmonic phonon model that describes the response of the system to a pulsed optical excitation. We find that the trilinear coupling of two orthogonal infrared-active phonons to a Raman-active phonon causes a transient distortion of the lattice. In contrast to the quadratic-linear coupling that has been previously explored, the direction of the distortion is determined by the polarization of the exciting light, introducing a novel mechanism for nonlinear phononic switching. Since the occurrence of the coupling is determined by the symmetry of the system we propose that it is a universal feature of orthorhombic and tetragonal perovskites.
Phonon triggered rhombohedral lattice distortion in vanadium at high pressure
Antonangeli, Daniele; Farber, Daniel L.; Bosak, Alexei; Aracne, Chantel M.; Ruddle, David G.; Krisch, Michael
2016-08-19
In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Lastly, our results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V.
Phonon triggered rhombohedral lattice distortion in vanadium at high pressure.
Antonangeli, Daniele; Farber, Daniel L; Bosak, Alexei; Aracne, Chantel M; Ruddle, David G; Krisch, Michael
2016-08-19
In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Our results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V.
Phonon triggered rhombohedral lattice distortion in vanadium at high pressure
Antonangeli, Daniele; Farber, Daniel L.; Bosak, Alexei; ...
2016-08-19
In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Lastly, ourmore » results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V.« less
Phonon triggered rhombohedral lattice distortion in vanadium at high pressure
Antonangeli, Daniele; Farber, Daniel L.; Bosak, Alexei; Aracne, Chantel M.; Ruddle, David G.; Krisch, Michael
2016-01-01
In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Our results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V. PMID:27539662
Yan, Zhequan; Chen, Liang; Yoon, Mina; ...
2016-01-12
Hexagonal boron nitride (h-BN) is a substrate for graphene based nano-electronic devices. We investigate the ballistic phonon transport at the interface of vertically stacked graphene and h-BN heterostructures using first principles density functional theory and atomistic Green's function simulations considering the influence of lattice stacking. We compute the frequency and wave-vector dependent transmission function and observe distinct stacking-dependent phonon transmission features for the h-BN/graphene/h-BN sandwiched systems. We find that the in-plane acoustic modes have the dominant contributions to the phonon transmission and thermal boundary conductance (TBC) for the interfaces with the carbon atom located directly on top of the boronmore » atom (C–B matched) because of low interfacial spacing. The low interfacial spacing is a consequence of the differences in the effective atomic volume of N and B and the difference in the local electron density around N and B. For the structures with the carbon atom directly on top of the nitrogen atom (C–N matched), the spatial distance increases and the contribution of in-plane modes to the TBC decreases leading to higher contributions by out-of-plane acoustic modes. We find that the C–B matched interfaces have stronger phonon–phonon coupling than the C–N matched interfaces, which results in significantly higher TBC (more than 50%) in the C–B matched interface. The findings in this study will provide insights to understand the mechanism of phonon transport at h-BN/graphene/h-BN interfaces, to better explain the experimental observations and to engineer these interfaces to enhance heat dissipation in graphene based electronic devices.« less
Yan, Zhequan; Chen, Liang; Yoon, Mina; Kumar, Satish
2016-01-12
Hexagonal boron nitride (h-BN) is a substrate for graphene based nano-electronic devices. We investigate the ballistic phonon transport at the interface of vertically stacked graphene and h-BN heterostructures using first principles density functional theory and atomistic Green's function simulations considering the influence of lattice stacking. We compute the frequency and wave-vector dependent transmission function and observe distinct stacking-dependent phonon transmission features for the h-BN/graphene/h-BN sandwiched systems. We find that the in-plane acoustic modes have the dominant contributions to the phonon transmission and thermal boundary conductance (TBC) for the interfaces with the carbon atom located directly on top of the boron atom (C–B matched) because of low interfacial spacing. The low interfacial spacing is a consequence of the differences in the effective atomic volume of N and B and the difference in the local electron density around N and B. For the structures with the carbon atom directly on top of the nitrogen atom (C–N matched), the spatial distance increases and the contribution of in-plane modes to the TBC decreases leading to higher contributions by out-of-plane acoustic modes. We find that the C–B matched interfaces have stronger phonon–phonon coupling than the C–N matched interfaces, which results in significantly higher TBC (more than 50%) in the C–B matched interface. The findings in this study will provide insights to understand the mechanism of phonon transport at h-BN/graphene/h-BN interfaces, to better explain the experimental observations and to engineer these interfaces to enhance heat dissipation in graphene based electronic devices.
Electron-Phonon Scattering in Atomically Thin 2D Perovskites.
Guo, Zhi; Wu, Xiaoxi; Zhu, Tong; Zhu, Xiaoyang; Huang, Libai
2016-11-22
Two-dimensional (2D) atomically thin perovskites with strongly bound excitons are highly promising for optoelectronic applications. However, the nature of nonradiative processes that limit the photoluminescence (PL) efficiency remains elusive. Here, we present time-resolved and temperature-dependent PL studies to systematically address the intrinsic exciton relaxation pathways in layered (C4H9NH3)2(CH3NH3)n-1PbnI3n+1 (n = 1, 2, 3) structures. Our results show that scatterings via deformation potential by acoustic and homopolar optical phonons are the main scattering mechanisms for excitons in ultrathin single exfoliated flakes, exhibiting a T(γ) (γ = 1.3 to 1.9) temperature dependence for scattering rates. We attribute the absence of polar optical phonon and defect scattering to efficient screening of Coulomb potential, similar to what has been observed in 3D perovskites. These results establish an understanding of the origins of nonradiative pathways and provide guidelines for optimizing PL efficiencies of atomically thin 2D perovskites.
NASA Technical Reports Server (NTRS)
Defacio, B.; Vannevel, Alan; Brander, O.
1993-01-01
A formulation is given for a collection of phonons (sound) in a fluid at a non-zero temperature which uses the simple harmonic oscillator twice; one to give a stochastic thermal 'noise' process and the other which generates a coherent Glauber state of phonons. Simple thermodynamic observables are calculated and the acoustic two point function, 'contrast' is presented. The role of 'coherence' in an equilibrium system is clarified by these results and the simple harmonic oscillator is a key structure in both the formulation and the calculations.
Abernathy, Douglas L.; Ma, Jie; Yan, Jiaqiang; Delaire, Olivier A.; Chen, Xi; Weathers, Annie; Mukhopadhyay, Saikat; Shi, Li
2015-04-15
A variety of crystals contain quasi-one-dimensional substructures, which yield distinctive electronic, spintronic, optical and thermoelectric properties. There is a lack of understanding of the lattice dynamics that influences the properties of such complex crystals. Here we employ inelastic neutron scatting measurements and density functional theory calculations to show that numerous low-energy optical vibrational modes exist in higher manganese silicides, an example of such crystals. These optical modes, including unusually low-frequency twisting motions of the Si ladders inside the Mn chimneys, provide a large phase space for scattering acoustic phonons. A hybrid phonon and diffuson model is proposed to explain the low and anisotropic thermal conductivity of higher manganese silicides and to evaluate nanostructuring as an approach to further suppress the thermal conductivity and enhance the thermoelectric energy conversion efficiency. This discovery offers new insights into the structure-property relationships of a broad class of materials with quasi-one-dimensional substructures for various applications.
An ultrawide-bandwidth single-sideband modulator for terahertz frequencies
NASA Astrophysics Data System (ADS)
Meijer, A. S.; Berden, G.; Arslanov, D. D.; Ozerov, M.; Jongma, R. T.; van der Zande, W. J.
2016-11-01
Wireless high-speed data communication using terahertz (THz) carrier frequencies is becoming reality with data rates beyond 100 Gbit s-1. Many of the mobile applications use internet access and require that THz wireless base stations are connected to a global network, such as the radio-over-fibre network. We present the realization of an ultrawide bandwidth THz optical single-sideband (OSSB) modulator for converting (free-space) THz signals to THz optical modulations with an increased spectral efficiency. THz OSSB will mitigate chromatic dispersion-induced propagation losses in optical fibres and support digital modulation schemes. We demonstrate THz OSSB for free-space radiation between 0.3 and 1.0 THz using a specially designed dichroic beamsplitter for signal and carrier, and a planar light-wave circuit with multimode interference structures. This arrangement of optical elements mimics the Hartley single-sideband modulator for electronics signals and accomplishes the required Hilbert transform without any frequency-dependent tuning element over an ultrawide THz spectrum.
Measurements of the ponderomotive force including sideband mode coupling effects and damping rates
Meassick, S.; Intrator, T.; Hershkowitz, N.; Browning, J.; Majeski, R.
1989-05-01
Measurements of the interactions of waves in the ion cyclotron range of frequencies (ICRF) with flute interchange modes are presented. Interactions between the applied l = 1 radio frequency (rf) wave and an m = -1 flute mode give rise to sidebands above and below the rf frequency with mode numbers of l = 0 and l = +2, respectively. The contribution of the sideband terms to stability are shown to cancel 40% of the direct ponderomotive contribution. This is less than the 90% predicted by theory (Phys. Fluids 30, 148 (1987)) for an applied l = +1 rf wave above the ion cyclotron frequency with a large separation between the plasma and the vacuum vessel. Measurements of the linear growth and damping rate of the flute instability in the presence of rf are in good agreement with that calculated by considering only the curvature-driven instability and the ponderomotive force. The growth rate of the magnetohydrodynamic mode is consistent with the primary force acting on the plasma being the curvature force. This method allows a determination of the net stabilizing force on the plasma.
Non-local effects in dual-probe-sideband Brillouin optical time domain analysis.
Dominguez-Lopez, Alejandro; Angulo-Vinuesa, Xabier; Lopez-Gil, Alexia; Martin-Lopez, Sonia; Gonzalez-Herraez, Miguel
2015-04-20
According to recent models, non-local effects in dual-probe-sideband Brillouin Optical Time Domain Analysis (BOTDA) systems should be essentially negligible whenever the probe power is below the Stimulated Brillouin Scattering (SBS) threshold. This paper shows that actually there appear non-local effects in this type of systems before the SBS threshold. To explain these effects it is necessary to take into account a full spectral description of the SBS process. The pump pulse experiences a frequency-dependent spectral deformation that affects the readout process differently in the gain and loss configurations. This paper provides a simple analytical model of this phenomenon, which is validated against compelling experimental data, showing good agreement. The main conclusion of our study is that the measurements in gain configuration are more robust to this non-local effect than the loss configuration. Experimental and theoretical results show that, for a total probe wave power of ~1 mW (500 μW on each sideband), there is an up-shifting of ~1 MHz in the Brillouin Frequency Shift (BFS) retrieved from the Brillouin Loss Spectrum, whereas the BFS extracted from the measured Brillouin Gain Spectrum is up-shifted only ~0.6 MHz. These results are of particular interest for manufacturers of long-range BOTDA systems.
Kumar, Naveen; Hatsagortsyan, Karen Z; Keitel, Christoph H
2013-09-06
Stimulated Raman scattering of an ultraintense laser pulse in plasmas is studied by perturbatively including the leading order term of the Landau-Lifshitz radiation reaction force in the equation of motion for plasma electrons. In this approximation, the radiation reaction force causes a phase shift in nonlinear current densities that drive the two Raman sidebands (anti-Stokes and Stokes waves), manifesting itself into the nonlinear mixing of two sidebands. This mixing results in a strong enhancement in the growth of the forward Raman scattering instability.
Phonovoltaic. III. Electron-phonon coupling and figure of merit of graphene:BN
NASA Astrophysics Data System (ADS)
Melnick, Corey; Kaviany, Massoud
2016-12-01
The phonovoltaic cell harvests optical phonons like a photovoltaic harvests photons, that is, a nonequilibrium (hot) population of optical phonons (at temperature Tp ,O) more energetic than the band gap produces electron-hole pairs in a p -n junction, which separates these pairs to produce power. A phonovoltaic material requires an optical phonon mode more energetic than its band gap and much more energetic than the thermal energy (Ep ,O>Δ Ee ,g≫kBT ), which relaxes by generating electrons and power (at rate γ˙e -p) rather than acoustic phonons and heat (at rate γ˙p -p). Graphene (h-C) is the most promising material candidate: when its band gap is tuned to its optical phonon energy without greatly reducing the electron-phonon (e -p ) coupling, it reaches a substantial figure of merit [ZpV=Δ Ee ,gγ˙e -p/Ep ,O(γ˙e -p+γ˙p -p) ≈0.8 ] . A simple tight-binding (TB) model presented here predicts that lifting the sublattice symmetry of graphene in order to open a band gap proscribes the e -p interaction at the band edge, such that γ˙e -p→0 as Δ Ee ,g→Ep ,O . However, ab initio (DFT-LDA) simulations of layered h-C/BN and substitutional h-C:BN show that the e -p coupling remains substantial in these asymmetric crystals. Indeed, h-C:BN achieves a high figure of merit (ZpV≈0.6 ). At 300 K and for a Carnot limit of 0.5 (Tp ,O=600 K) , a h-C:BN phonovoltaic can reach an efficiency of ηpV≈0.2 , double the thermoelectric efficiency (Z T ≈1 ) under similar conditions.
Flow stabilization by subsurface phonons
Hussein, M. I.; Biringen, S.; Bilal, O. R.; Kucala, A.
2015-01-01
The interaction between a fluid and a solid surface in relative motion represents a dynamical process that is central to the problem of laminar-to-turbulent transition (and consequent drag increase) for air, sea and land vehicles, as well as long-range pipelines. This problem may in principle be alleviated via a control stimulus designed to impede the generation and growth of instabilities inherent in the flow. Here, we show that phonon motion underneath a surface may be tuned to passively generate a spatio-temporal elastic deformation profile at the surface that counters these instabilities. We theoretically demonstrate this phenomenon and the underlying mechanism of frequency-dependent destructive interference of the unstable flow waves. The converse process of flow destabilization is illustrated as well. This approach provides a condensed-matter physics treatment to fluid–structure interaction and a new paradigm for flow control. PMID:27547095
Two-Dimensional Phononic Crystals: Disorder Matters.
Wagner, Markus R; Graczykowski, Bartlomiej; Reparaz, Juan Sebastian; El Sachat, Alexandros; Sledzinska, Marianna; Alzina, Francesc; Sotomayor Torres, Clivia M
2016-09-14
The design and fabrication of phononic crystals (PnCs) hold the key to control the propagation of heat and sound at the nanoscale. However, there is a lack of experimental studies addressing the impact of order/disorder on the phononic properties of PnCs. Here, we present a comparative investigation of the influence of disorder on the hypersonic and thermal properties of two-dimensional PnCs. PnCs of ordered and disordered lattices are fabricated of circular holes with equal filling fractions in free-standing Si membranes. Ultrafast pump and probe spectroscopy (asynchronous optical sampling) and Raman thermometry based on a novel two-laser approach are used to study the phononic properties in the gigahertz (GHz) and terahertz (THz) regime, respectively. Finite element method simulations of the phonon dispersion relation and three-dimensional displacement fields furthermore enable the unique identification of the different hypersonic vibrations. The increase of surface roughness and the introduction of short-range disorder are shown to modify the phonon dispersion and phonon coherence in the hypersonic (GHz) range without affecting the room-temperature thermal conductivity. On the basis of these findings, we suggest a criteria for predicting phonon coherence as a function of roughness and disorder.
Acoustically trapped colloidal crystals that are reconfigurable in real time.
Caleap, Mihai; Drinkwater, Bruce W
2014-04-29
Photonic and phononic crystals are metamaterials with repeating unit cells that result in internal resonances leading to a range of wave guiding and filtering properties and are opening up new applications such as hyperlenses and superabsorbers. Here we show the first, to our knowledge, 3D colloidal phononic crystal that is reconfigurable in real time and demonstrate its ability to rapidly alter its frequency filtering characteristics. Our reconfigurable material is assembled from microspheres in aqueous solution, trapped with acoustic radiation forces. The acoustic radiation force is governed by an energy landscape, determined by an applied high-amplitude acoustic standing wave field, in which particles move swiftly to energy minima. This creates a colloidal crystal of several milliliters in volume with spheres arranged in an orthorhombic lattice in which the acoustic wavelength is used to control the lattice spacing. Transmission acoustic spectroscopy shows that the new colloidal crystal behaves as a phononic metamaterial and exhibits clear band-pass and band-stop frequencies which are adjusted in real time.
Balram, Krishna C; Davanço, Marcelo I; Song, Jin Dong; Srinivasan, Kartik
2016-05-01
Optomechanical cavities have been studied for applications ranging from sensing to quantum information science. Here, we develop a platform for nanoscale cavity optomechanical circuits in which optomechanical cavities supporting co-localized 1550 nm photons and 2.4 GHz phonons are combined with photonic and phononic waveguides. Working in GaAs facilitates manipulation of the localized mechanical mode either with a radio frequency (RF) field through the piezo-electric effect, which produces acoustic waves that are routed and coupled to the optomechanical cavity by phononic crystal waveguides, or optically through the strong photoelastic effect. Along with mechanical state preparation and sensitive readout, we use this to demonstrate an acoustic wave interference effect, similar to atomic coherent population trapping, in which RF-driven coherent mechanical motion is cancelled by optically-driven motion. Manipulating cavity optomechanical systems with equal facility through both photonic and phononic channels enables new architectures for signal transduction between the optical, electrical, and mechanical domains.
NASA Astrophysics Data System (ADS)
Basu, A.; Das, B.; Middya, T. R.; Bhattacharya, D. P.
2017-01-01
The phonon growth characteristic in a degenerate semiconductor has been calculated under the condition of low temperature. If the lattice temperature is high, the energy of the intravalley acoustic phonon is negligibly small compared to the average thermal energy of the electrons. Hence one can traditionally assume the electron-phonon collisions to be elastic and approximate the Bose-Einstein (B.E.) distribution for the phonons by the simple equipartition law. However, in the present analysis at the low lattice temperatures, the interaction of the non equilibrium electrons with the acoustic phonons becomes inelastic and the simple equipartition law for the phonon distribution is not valid. Hence the analysis is made taking into account the inelastic collisions and the complete form of the B.E. distribution. The high-field distribution function of the carriers given by Fermi-Dirac (F.D.) function at the field dependent carrier temperature, has been approximated by a well tested model that apparently overcomes the intrinsic problem of correct evaluation of the integrals involving the product and powers of the Fermi function. Hence the results thus obtained are more reliable compared to the rough estimation that one may obtain from using the exact F.D. function, but taking recourse to some over simplified approximations.
Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe_{1-x}M_{x}Si, M=Ir,Os
Delaire, O.; Al-Qasir, Iyad I.; May, Andrew F.; Sales, Brian C.; Niedziela, Jennifer L.; Ma, Jie; Matsuda, Masaaki; Abernathy, Douglas L.; Berlijn, Tom
2015-03-31
The vibrational behavior of heavy substitutional impurities (M=Ir,Os) in Fe_{1-x}M_{x}Si (x = 0, 0.02, 0.04, 0.1) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. In this paper, our INS measurements on single-crystals mapped the four-dimensional dynamical structure factor, S(Q;E), for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers and increases electron-phonon coupling, leads to softened interatomic force-constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S(Q,E) from INS through a Green's function model incorporating the phonon self-energy based on first-principles density functional theory (DFT) simulations. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Finally, our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.
Electron-phonon superconductivity in YIn3
NASA Astrophysics Data System (ADS)
Billington, D.; Llewellyn-Jones, T. M.; Maroso, G.; Dugdale, S. B.
2013-08-01
First-principles calculations of the electron-phonon coupling were performed on the cubic intermetallic compound YIn3. The electron-phonon coupling constant was found to be λep = 0.42. Using the Allen-Dynes formula with a Coulomb pseudopotential of μ* = 0.10, a Tc of approximately 0.77 K is obtained which is reasonably consistent with the experimentally observed temperature (between 0.8 and 1.1 K). The results indicate that conventional electron-phonon coupling is capable of producing the superconductivity in this compound.
Electrons and Phonons in Semiconductor Multilayers
NASA Astrophysics Data System (ADS)
Ridley, B. K.
2014-08-01
Introduction; 1. Simple models of the electron-phonon interaction; 2. Quantum confinement of carriers; 3. Quasicontinuum theory of lattice vibrations; 4. Bulk vibratory modes in an isotropic continuum; 5. Optical modes in a quantum well; 6. Superlattice modes; 7. Optical modes in various structures; 8. Electron-phonon interaction in a quantum well; 9. Other scattering mechanisms; 10. Quantum screening; 11. The electron distribution function; 12. Spin relaxation; 13. Electrons and phonons in the Wurtzite lattice; 14. Nitride heterostructures; 15. Terahertz sources; References; Index.
NASA Astrophysics Data System (ADS)
Gough, Colin
This chapter provides an introduction to the physical and psycho-acoustic principles underlying the production and perception of the sounds of musical instruments. The first section introduces generic aspects of musical acoustics and the perception of musical sounds, followed by separate sections on string, wind and percussion instruments.
Size and temperature dependence of the electron-phonon scattering by donors in nanowire transistors
NASA Astrophysics Data System (ADS)
Bescond, M.; Carrillo-Nuñez, H.; Berrada, S.; Cavassilas, N.; Lannoo, M.
2016-08-01
Due to the constant size reduction, single-donor-based nanowire transistors receive an increasing interest from the semi-conductor industry. In this work we theoretically investigate the coupled influence of electron-phonon scattering, temperature and size (cross-section and channel length) on the properties of such systems. The aim is to determine under what conditions the localized character of the donor has a remarkable impact on the current characteristics. We use a quantum non-equilibrium Green's function approach in which the acoustic electron-phonon scattering is treated through local self-energies. We first show how this widely used approach, valid at high temperatures, can be extended to lower temperatures. Our simulations predict a hysteresis in the current when reducing the temperature down to 150 K. We also find that acoustic phonons degrade the current characteristics while their optical counterparts might have a beneficial impact with an increase of the ON-current. Finally we discuss the influence of nanowire length and cross-section and emphasize the complexity of precisely controlling the dopant level at room temperature.
Enhancing phonon flow through one-dimensional interfaces by impedance matching
Polanco, Carlos A. Ghosh, Avik W.
2014-08-28
We extend concepts from microwave engineering to thermal interfaces and explore the principles of impedance matching in 1D. The extension is based on the generalization of acoustic impedance to nonlinear dispersions using the contact broadening matrix Γ(ω), extracted from the phonon self energy. For a single junction, we find that for coherent and incoherent phonons, the optimal thermal conductance occurs when the matching Γ(ω) equals the Geometric Mean of the contact broadenings. This criterion favors the transmission of both low and high frequency phonons by requiring that (1) the low frequency acoustic impedance of the junction matches that of the two contacts by minimizing the sum of interfacial resistances and (2) the cut-off frequency is near the minimum of the two contacts, thereby reducing the spillage of the states into the tunneling regime. For an ultimately scaled single atom/spring junction, the matching criterion transforms to the arithmetic mean for mass and the harmonic mean for spring constant. The matching can be further improved using a composite graded junction with an exponential varying broadening that functions like a broadband antireflection coating. There is, however, a trade off as the increased length of the interface brings in additional intrinsic sources of scattering.
Morozovska, Anna N.; Vysochanskii, Yulian M.; Varenyk, Oleksandr V.; Silibin, Maxim V.; Kalinin, Sergei V.; Eliseev, Eugene A.
2015-09-29
The impact of the flexoelectric effect on the generalized susceptibility and soft phonon dispersion is not well known in the long-range-ordered phases of ferroics. Within the Landau-Ginzburg-Devonshire approach we obtained analytical expressions for the generalized susceptibility and phonon dispersion relations in the ferroelectric phase. The joint action of the static and dynamic flexoelectric effects induces nondiagonal components of the generalized susceptibility, whose amplitude is proportional to the convolution of the spontaneous polarization with the flexocoupling constants. The flexocoupling essentially broadens the k spectrum of the generalized susceptibility and leads to an additional “pushing away” of the optical and acoustic soft mode phonon branches. The degeneracy of the transverse optical and acoustic modes disappears in the ferroelectric phase in comparison with the paraelectric phase due to the joint action of flexoelectric coupling and ferroelectric nonlinearity. Lastly, the results obtained might be mainly important for theoretical analyses of a broad spectrum of experimental data, including neutron and Brillouin scattering.
Morozovska, Anna N.; Vysochanskii, Yulian M.; Varenyk, Oleksandr V.; ...
2015-09-29
The impact of the flexoelectric effect on the generalized susceptibility and soft phonon dispersion is not well known in the long-range-ordered phases of ferroics. Within the Landau-Ginzburg-Devonshire approach we obtained analytical expressions for the generalized susceptibility and phonon dispersion relations in the ferroelectric phase. The joint action of the static and dynamic flexoelectric effects induces nondiagonal components of the generalized susceptibility, whose amplitude is proportional to the convolution of the spontaneous polarization with the flexocoupling constants. The flexocoupling essentially broadens the k spectrum of the generalized susceptibility and leads to an additional “pushing away” of the optical and acoustic softmore » mode phonon branches. The degeneracy of the transverse optical and acoustic modes disappears in the ferroelectric phase in comparison with the paraelectric phase due to the joint action of flexoelectric coupling and ferroelectric nonlinearity. Lastly, the results obtained might be mainly important for theoretical analyses of a broad spectrum of experimental data, including neutron and Brillouin scattering.« less
Control of coherent information via on-chip photonic-phononic emitter-receivers.
Shin, Heedeuk; Cox, Jonathan A; Jarecki, Robert; Starbuck, Andrew; Wang, Zheng; Rakich, Peter T
2015-03-05
Rapid progress in integrated photonics has fostered numerous chip-scale sensing, computing and signal processing technologies. However, many crucial filtering and signal delay operations are difficult to perform with all-optical devices. Unlike photons propagating at luminal speeds, GHz-acoustic phonons moving at slower velocities allow information to be stored, filtered and delayed over comparatively smaller length-scales with remarkable fidelity. Hence, controllable and efficient coupling between coherent photons and phonons enables new signal processing technologies that greatly enhance the performance and potential impact of integrated photonics. Here we demonstrate a mechanism for coherent information processing based on travelling-wave photon-phonon transduction, which achieves a phonon emit-and-receive process between distinct nanophotonic waveguides. Using this device, physics--which supports GHz frequencies--we create wavelength-insensitive radiofrequency photonic filters with frequency selectivity, narrow-linewidth and high power-handling in silicon. More generally, this emit-receive concept is the impetus for enabling new signal processing schemes.
Optic phonons and anisotropic thermal conductivity in hexagonal Ge2Sb2Te5
Mukhopadhyay, Saikat; Lindsay, Lucas; Singh, David J.
2016-01-01
The lattice thermal conductivity (κ) of hexagonal Ge2Sb2Te5 (h-GST) is studied via direct first-principles calculations. We find significant intrinsic anisotropy (κa/κc~2) of κ in bulk h-GST, with the dominant contribution to κ from optic phonons, ~75%. This is extremely unusual as the acoustic phonon modes are the majority heat carriers in typical semiconductors and insulators. The anisotropy derives from varying bonding along different crystal directions, specifically from weak interlayer bonding along the c-axis, which gives anisotropic phonon dispersions. The phonon spectrum of h-GST has very dispersive optic branches with higher group velocities along the a-axis as compared to flat optic bands along the c-axis. The large optic mode contributions to the thermal conductivity in low-κ h-GST is unusual, and development of fundamental physical understanding of these contributions may be critical to better understanding of thermal conduction in other complex layered materials. PMID:27848985
Control of coherent information via on-chip photonic–phononic emitter–receivers
Shin, Heedeuk; Cox, Jonathan A.; Jarecki, Robert; Starbuck, Andrew; Wang, Zheng; Rakich, Peter T.
2015-01-01
Rapid progress in integrated photonics has fostered numerous chip-scale sensing, computing and signal processing technologies. However, many crucial filtering and signal delay operations are difficult to perform with all-optical devices. Unlike photons propagating at luminal speeds, GHz-acoustic phonons moving at slower velocities allow information to be stored, filtered and delayed over comparatively smaller length-scales with remarkable fidelity. Hence, controllable and efficient coupling between coherent photons and phonons enables new signal processing technologies that greatly enhance the performance and potential impact of integrated photonics. Here we demonstrate a mechanism for coherent information processing based on travelling-wave photon–phonon transduction, which achieves a phonon emit-and-receive process between distinct nanophotonic waveguides. Using this device, physics—which supports GHz frequencies—we create wavelength-insensitive radiofrequency photonic filters with frequency selectivity, narrow-linewidth and high power-handling in silicon. More generally, this emit-receive concept is the impetus for enabling new signal processing schemes. PMID:25740405
Effects of vacancies on phonon entropy of B2 FeAl
Lucas, M.S.; Delaire, O.; Winterrose, M.L.; Swan-Wood, T.; Kresch, M.; Halevy, I.; Fultz, B.; Hu, Jingzhu; Lerche, M.; Hu, M.Y.; Somayazulu, M.; CIT; ORNL; CIW; UC
2010-01-12
The phonon density of states (DOS) and phonon entropy of B2 FeAl were determined as functions of the Fe site vacancy concentration using several scattering techniques and were computed from first principles. Measurements at elevated temperature and pressure were performed to explore volume effects, test the usefulness of the quasiharmonic (QH) approximation, and provide comparison for the first-principles calculations. The average temperature and pressure dependencies of phonons were consistent with the QH model. The decrease in specific volume associated with the introduction of vacancies causes a stiffening of the DOS that was captured well with the experimentally determined Grueneisen parameter. Features associated with vacancies in the DOS are not well explained by this model, however, especially in the gap between the acoustic and optic branches. First-principles calculations indicated that these modes are primarily associated with vibrations of Al atoms in the first-nearest-neighbor shell of the vacancy, with some vibration amplitude also involving the second-nearest-neighbor Fe atoms. At the vacancy concentrations of study, the phonon entropy of vacancy formation was found to be approximately -1.7k{sub B}/atom, about half as large and of opposite sign as the configurational entropy of vacancy formation.
Control of coherent information via on-chip photonic–phononic emitter–receivers
Shin, Heedeuk; Cox, Jonathan A.; Jarecki, Robert; Starbuck, Andrew; Wang, Zheng; Rakich, Peter T.
2015-03-05
We report that rapid progress in integrated photonics has fostered numerous chip-scale sensing, computing and signal processing technologies. However, many crucial filtering and signal delay operations are difficult to perform with all-optical devices. Unlike photons propagating at luminal speeds, GHz-acoustic phonons moving at slower velocities allow information to be stored, filtered and delayed over comparatively smaller length-scales with remarkable fidelity. Hence, controllable and efficient coupling between coherent photons and phonons enables new signal processing technologies that greatly enhance the performance and potential impact of integrated photonics. Here we demonstrate a mechanism for coherent information processing based on travelling-wave photon–phonon transduction, which achieves a phonon emit-and-receive process between distinct nanophotonic waveguides. Using this device, physics—which supports GHz frequencies—we create wavelength-insensitive radiofrequency photonic filters with frequency selectivity, narrow-linewidth and high power-handling in silicon. More generally, this emit-receive concept is the impetus for enabling new signal processing schemes.
Control of coherent information via on-chip photonic–phononic emitter–receivers
Shin, Heedeuk; Cox, Jonathan A.; Jarecki, Robert; ...
2015-03-05
We report that rapid progress in integrated photonics has fostered numerous chip-scale sensing, computing and signal processing technologies. However, many crucial filtering and signal delay operations are difficult to perform with all-optical devices. Unlike photons propagating at luminal speeds, GHz-acoustic phonons moving at slower velocities allow information to be stored, filtered and delayed over comparatively smaller length-scales with remarkable fidelity. Hence, controllable and efficient coupling between coherent photons and phonons enables new signal processing technologies that greatly enhance the performance and potential impact of integrated photonics. Here we demonstrate a mechanism for coherent information processing based on travelling-wave photon–phonon transduction,more » which achieves a phonon emit-and-receive process between distinct nanophotonic waveguides. Using this device, physics—which supports GHz frequencies—we create wavelength-insensitive radiofrequency photonic filters with frequency selectivity, narrow-linewidth and high power-handling in silicon. More generally, this emit-receive concept is the impetus for enabling new signal processing schemes.« less
Optic phonons and anisotropic thermal conductivity in hexagonal Ge2Sb2Te5
NASA Astrophysics Data System (ADS)
Mukhopadhyay, Saikat; Lindsay, Lucas; Singh, David J.
2016-11-01
The lattice thermal conductivity (κ) of hexagonal Ge2Sb2Te5 (h-GST) is studied via direct first-principles calculations. We find significant intrinsic anisotropy (κa/κc~2) of κ in bulk h-GST, with the dominant contribution to κ from optic phonons, ~75%. This is extremely unusual as the acoustic phonon modes are the majority heat carriers in typical semiconductors and insulators. The anisotropy derives from varying bonding along different crystal directions, specifically from weak interlayer bonding along the c-axis, which gives anisotropic phonon dispersions. The phonon spectrum of h-GST has very dispersive optic branches with higher group velocities along the a-axis as compared to flat optic bands along the c-axis. The large optic mode contributions to the thermal conductivity in low-κ h-GST is unusual, and development of fundamental physical understanding of these contributions may be critical to better understanding of thermal conduction in other complex layered materials.
Optic phonons and anisotropic thermal conductivity in hexagonal Ge2Sb2Te5
Mukhopadhyay, Saikat; Lindsay, Lucas R.; Singh, David
2016-11-16
The lattice thermal conductivity ($κ$) of hexagonal Ge2Sb2Tesub>5 (h-GST) is studied via direct first-principles calculations. We find significant intrinsic anisotropy of ( $κ$a/$κ$c~2) of $κ$ in bulk h-GST along different transport directions. The dominant contribution to$κ$ is from optic phonons, ~75%. This is extremely unusual as the acoustic phonon modes carry most of the heat in typical semiconductors and insulators with small unit cells. Very recently, Lee et. al. observed anisotropic in GST thin films and attributed this to thermal resistance of amorphous regions near grain boundaries. However, our results suggest an additional strong intrinsic anisotropy for the pure hexagonalmore » phase. This derives from bonding anisotropy along different crystal directions, specifically from weak interlayer coupling, which gives anisotropic phonon dispersions. The phonon spectrum of h-GST has very dispersive optic branches with higher group velocities along the a-axis as compared to flat optic bands along the c-axis. The importance of optic mode contributions for the thermal conductivity in low-$κ$ h-GST is unusual, and development of fundamental physical understanding of these contributions may be critical to better understanding of thermal conduction in other complex layered materials.« less
Hawking Radiation from an Acoustic Black Hole on an Ion Ring
Horstmann, B.; Cirac, J. I.; Reznik, B.; Fagnocchi, S.
2010-06-25
In this Letter we propose to simulate acoustic black holes with ions in rings. If the ions are rotating with a stationary and inhomogeneous velocity profile, regions can appear where the ion velocity exceeds the group velocity of the phonons. In these regions phonons are trapped like light in black holes, even though we have a discrete field theory and a nonlinear dispersion relation. We study the appearance of Hawking radiation in this setup and propose a scheme to detect it.
Electron-phonon superconductivity in BaSn5
NASA Astrophysics Data System (ADS)
Billington, David; Ernsting, David; Millichamp, Thomas E.; Dugdale, Stephen B.
2015-05-01
First-principles calculations of the electronic structure and phonon dispersion relation of the superconducting compound ? were performed. This has allowed the calculation of the electron-phonon matrix elements from which the electron-phonon coupling constant was found to be ?. Application of the Allen-Dynes formula with ? yielded a superconducting transition temperature of ? K. The calculated ? agrees well with the available experimental data and indicates that ? is an electron-phonon superconductor with intermediate strength electron-phonon coupling.
Parsons, L. C. Andrews, G. T.
2014-07-21
Brillouin light scattering experiments and optical reflectance measurements were performed on a pair of porous silicon-based optical Bragg mirrors which had constituent layer porosity ratios close to unity. For off-axis propagation, the phononic and photonic band structures of the samples were modeled as a series of intersecting linear dispersion curves. Zone-folding was observed for the longitudinal bulk acoustic phonon and the frequency of the probed zone-folded longitudinal phonon was shown to be dependent on the propagation direction as well as the folding order of the mode branch. There was no conclusive evidence of coupling between the transverse and the folded longitudinal modes. Two additional observed Brillouin peaks were attributed to the Rayleigh surface mode and a possible pseudo-surface mode. Both of these modes were dispersive, with the velocity increasing as the wavevector decreased.
Stationary Phonon Squeezing by Optical Polaron Excitation
NASA Astrophysics Data System (ADS)
Papenkort, T.; Axt, V. M.; Kuhn, T.
2017-03-01
We demonstrate that a stationary squeezed phonon state can be prepared by a pulsed optical excitation of a semiconductor quantum well. Unlike previously discussed scenarios for generating squeezed phonons, the corresponding uncertainties become stationary after the excitation and do not oscillate in time. The effect is caused by two-phonon correlations within the excited polaron. We demonstrate by quantum kinetic simulations and by a perturbation analysis that the energetically lowest polaron state comprises two-phonon correlations which, after the pulse, result in an uncertainty of the lattice momentum that is continuously lower than in the ground state of the semiconductor. The simulations show the dynamics of the polaron formation process and the resulting time-dependent lattice uncertainties.
Nanoscale pillar hypersonic surface phononic crystals
NASA Astrophysics Data System (ADS)
Yudistira, D.; Boes, A.; Graczykowski, B.; Alzina, F.; Yeo, L. Y.; Sotomayor Torres, C. M.; Mitchell, A.
2016-09-01
We report on nanoscale pillar-based hypersonic phononic crystals in single crystal Z-cut lithium niobate. The phononic crystal is formed by a two-dimensional periodic array of nearly cylindrical nanopillars 240 nm in diameter and 225 nm in height, arranged in a triangular lattice with a 300-nm lattice constant. The nanopillars are fabricated by the recently introduced nanodomain engineering via laser irradiation of patterned chrome followed by wet etching. Numerical simulations and direct measurements using Brillouin light scattering confirm the simultaneous existence of nonradiative complete surface phononic band gaps. The band gaps are found below the sound line at hypersonic frequencies in the range 2-7 GHz, formed from local resonances and Bragg scattering. These hypersonic structures are realized directly in the piezoelectric material lithium niobate enabling phonon manipulation at significantly higher frequencies than previously possible with this platform, opening new opportunities for many applications in plasmonic, optomechanic, microfluidic, and thermal engineering.
Phonon stop bands in amorphous superlattices
NASA Astrophysics Data System (ADS)
Koblinger, O.; Mebert, J.; Dittrich, E.; Döttinger, S.; Eisenmenger, W.; Santos, P. V.; Ley, L.
1987-06-01
In periodically layered media the phonon-dispersion relation shows energy ranges in which phonon propagation is not possible. The existence of such phonon stop bands in crystalline superlattices has been observed in work by V. Narayanamurti, H. L. Störmer, M. A. Chin, A. C. Gossard, and W. Wiegman [Phys. Rev. Lett. 43, 2012 (1979)]. In this Communication we report the observation of phonon stop bands in amorphous superlattices. The filter characteristic of these amorphous superlattices is much sharper than in the case of the crystalline superlattices studied earlier. The investigated superlattices have been prepared by alternating evaporation of Si and SiO2 layers as well as by plasma-enhanced chemical vapor deposition of a-Si:H/a-SiNx:H films in a glow-discharge reactor.
Parshall, D.; Pintschovius, L.; Niedziela, Jennifer L.; ...
2015-04-27
Pmore » arent compounds of Fe-based superconductors undergo a structural phase transition from a tetragonal to an orthorhombic structure. We investigated the temperature dependence of the frequencies of TA phonons that extrapolate to the shear vibrational mode at the zone center, which corresponds to the orthorhombic deformation of the crystal structure at low temperatures in BaFe2As2 and SrFe2As2. We found that acoustic phonons at small wave vectors soften gradually towards the transition from high temperatures, tracking the increase of the size of slowly fluctuating magnetic domains. On cooling below the transition to base temperature the phonons harden, following the square of the magnetic moment (which we find is proportional to the anisotropy gap). Finally, our results provide evidence for close correlation between magnetic and phonon properties in Fe-based superconductors.« less
Code of Federal Regulations, 2010 CFR
2010-10-01
... 47 Telecommunication 4 2010-10-01 2010-10-01 false System specifications for double-sideband (DBS) modulated emissions in the HF broadcasting service. 73.756 Section 73.756 Telecommunication FEDERAL... broadcasting service. (a) Channel spacing. The nominal spacing for DSB shall be 10 kHz. However,...
Phonon Cooling by an Optomechanical Heat Pump.
Dong, Ying; Bariani, F; Meystre, P
2015-11-27
We propose and analyze theoretically a cavity optomechanical analog of a heat pump that uses a polariton fluid to cool mechanical modes coupled to a single precooled phonon mode via external modulation of the substrate of the mechanical resonator. This approach permits us to cool phonon modes of arbitrary frequencies not limited by the cavity-optical field detuning deep into the quantum regime from room temperature.
Phonon Enhancement of Electronic and Optoelectronic Devices
2006-12-01
2 Task #1 Phonon Engineering for the Development of Terahertz Lasers Based On...terms of the MURI program highlights and outcome, the following merit special mention: (a) the project area involving Terahertz lasers (Task #1, led by...design an all-optical experiment on GHz range GaN /AIGaN FETs with considerable input from H. Maris (modulation spectroscopy; coherent phonon generation
NASA Astrophysics Data System (ADS)
Sundaresan, Sasi Sekaran
Monte Carlo based statistical approach to solve Boltzmann Transport Equation (BTE) has become a norm to investigate heat transport in semiconductors at sub-micron regime, owing mainly to its ability to characterize realistically sized device geometries qualitatively. One of the primary issues with this technique is that the approach predominantly uses empirically fitted phonon dispersion relations as input to determine the properties of phonons so as to predict the thermal conductivity of specified material geometry. The empirically fitted dispersion relations assume harmonic approximation thereby failing to account for thermal expansion, interaction of lattice waves, effect of strain on spring stiffness, and accurate phonon-phonon interaction. To circumvent this problem, in this work, a coupled molecular mechanics-Monte Carlo (MM-MC) platform has been developed and used to solve the phonon Boltzmann Transport Equation (BTE) for the calculation of thermal conductivity of several novel and emerging nanostructures. The use of the quasi-anharmonic MM approach (as implemented in the open source NEMO 3-D software toolkit) not only allows one to capture the true atomicity of the underlying lattice but also enables the simulation of realistically-sized structures containing millions of atoms. As compared to the approach using an empirically fitted phonon dispersion relation, here, a 17% increase in the thermal conductivity for a silicon nanowire due to the incorporation of atomistic corrections in the LA (longitudinal acoustic) branch alone has been reported. The atomistically derived thermal conductivity as calculated from the MM-MC framework is then used in the modular design and analysis of (i) a silicon nanowire based thermoelectric cooler (TEC) unit, and (ii) a GaN/InN based nanostructured light emitting device (LED). It is demonstrated that the use of empirically fitted phonon bandstructure parameters overestimates the temperature difference between the hot and the
Toward quantitative modeling of silicon phononic thermocrystals
NASA Astrophysics Data System (ADS)
Lacatena, V.; Haras, M.; Robillard, J.-F.; Monfray, S.; Skotnicki, T.; Dubois, E.
2015-03-01
The wealth of technological patterning technologies of deca-nanometer resolution brings opportunities to artificially modulate thermal transport properties. A promising example is given by the recent concepts of "thermocrystals" or "nanophononic crystals" that introduce regular nano-scale inclusions using a pitch scale in between the thermal phonons mean free path and the electron mean free path. In such structures, the lattice thermal conductivity is reduced down to two orders of magnitude with respect to its bulk value. Beyond the promise held by these materials to overcome the well-known "electron crystal-phonon glass" dilemma faced in thermoelectrics, the quantitative prediction of their thermal conductivity poses a challenge. This work paves the way toward understanding and designing silicon nanophononic membranes by means of molecular dynamics simulation. Several systems are studied in order to distinguish the shape contribution from bulk, ultra-thin membranes (8 to 15 nm), 2D phononic crystals, and finally 2D phononic membranes. After having discussed the equilibrium properties of these structures from 300 K to 400 K, the Green-Kubo methodology is used to quantify the thermal conductivity. The results account for several experimental trends and models. It is confirmed that the thin-film geometry as well as the phononic structure act towards a reduction of the thermal conductivity. The further decrease in the phononic engineered membrane clearly demonstrates that both phenomena are cumulative. Finally, limitations of the model and further perspectives are discussed.
Toward quantitative modeling of silicon phononic thermocrystals
Lacatena, V.; Haras, M.; Robillard, J.-F. Dubois, E.; Monfray, S.; Skotnicki, T.
2015-03-16
The wealth of technological patterning technologies of deca-nanometer resolution brings opportunities to artificially modulate thermal transport properties. A promising example is given by the recent concepts of 'thermocrystals' or 'nanophononic crystals' that introduce regular nano-scale inclusions using a pitch scale in between the thermal phonons mean free path and the electron mean free path. In such structures, the lattice thermal conductivity is reduced down to two orders of magnitude with respect to its bulk value. Beyond the promise held by these materials to overcome the well-known “electron crystal-phonon glass” dilemma faced in thermoelectrics, the quantitative prediction of their thermal conductivity poses a challenge. This work paves the way toward understanding and designing silicon nanophononic membranes by means of molecular dynamics simulation. Several systems are studied in order to distinguish the shape contribution from bulk, ultra-thin membranes (8 to 15 nm), 2D phononic crystals, and finally 2D phononic membranes. After having discussed the equilibrium properties of these structures from 300 K to 400 K, the Green-Kubo methodology is used to quantify the thermal conductivity. The results account for several experimental trends and models. It is confirmed that the thin-film geometry as well as the phononic structure act towards a reduction of the thermal conductivity. The further decrease in the phononic engineered membrane clearly demonstrates that both phenomena are cumulative. Finally, limitations of the model and further perspectives are discussed.
From Modal Mixing to Tunable Functional Switches in Nonlinear Phononic Crystals
NASA Astrophysics Data System (ADS)
Ganesh, R.; Gonella, S.
2015-02-01
We introduce a paradigm for spatial and modal wave manipulation based on nonlinear phononic crystals and explore its potential for engineering wave control systems with tunable, adaptive, and multifunctional characteristics. Our approach exploits nonlinear mechanisms to stretch the frequency signature of the wave response and distribute it over multiple modes, thereby activating a mixture of modal characteristics and enabling functionalities associated with high-frequency optical modes, even while operating in the low-frequency regime. To elucidate the versatility of this approach, we consider different granular crystal configurations that span the available landscape of crystal topologies and wave control functionalities. The ability to switch between complementary functionalities allows rethinking nonlinear phononic crystals as programmable acoustic ports that form the building blocks of a new structural logic framework enabled by nonlinearity.
Phonon spectroscopy with sub-meV resolution by femtosecond x-ray diffuse scattering
Zhu, Diling; Robert, Aymeric; Henighan, Tom; ...
2015-08-10
We present a reconstruction of the transverse acoustic phonon dispersion of germanium from femtosecond time-resolved x-ray diffuse scattering measurements at the Linac Coherent Light Source. We demonstrate an energy resolution of 0.3 meV with a momentum resolution of 0.01 nm-1 using 10-keV x rays with a bandwidth of ~ 1 eV. This high resolution was achieved simultaneously for a large section of reciprocal space including regions closely following three of the principal symmetry directions. The phonon dispersion was reconstructed with less than 3 h of measurement time, during which neither the x-ray energy, the sample orientation, nor the detector positionmore » were scanned. In conclusion, these results demonstrate how time-domain measurements can complement conventional frequency domain inelastic-scattering techniques.« less
Orbital angular momentum mode division filtering for photon-phonon coupling
NASA Astrophysics Data System (ADS)
Zhu, Zhi-Han; Sheng, Li-Wen; Lv, Zhi-Wei; He, Wei-Ming; Gao, Wei
2017-01-01
Stimulated Brillouin scattering (SBS), a fundamental nonlinear interaction between light and acoustic waves occurring in any transparency material, has been broadly studied for several decades and gained rapid progress in integrated photonics recently. However, the SBS noise arising from the unwanted coupling between photons and spontaneous non-coherent phonons in media is inevitable. Here, we propose and experimentally demonstrate this obstacle can be overcome via a method called orbital angular momentum mode division filtering. Owing to the introduction of a new distinguishable degree-of-freedom, even extremely weak signals can be discriminated and separated from a strong noise produced in SBS processes. The mechanism demonstrated in this proof-of-principle work provides a practical way for quasi-noise-free photonic-phononic operation, which is still valid in waveguides supporting multi-orthogonal spatial modes, permits more flexibility and robustness for future SBS devices.
Orbital angular momentum mode division filtering for photon-phonon coupling.
Zhu, Zhi-Han; Sheng, Li-Wen; Lv, Zhi-Wei; He, Wei-Ming; Gao, Wei
2017-01-10
Stimulated Brillouin scattering (SBS), a fundamental nonlinear interaction between light and acoustic waves occurring in any transparency material, has been broadly studied for several decades and gained rapid progress in integrated photonics recently. However, the SBS noise arising from the unwanted coupling between photons and spontaneous non-coherent phonons in media is inevitable. Here, we propose and experimentally demonstrate this obstacle can be overcome via a method called orbital angular momentum mode division filtering. Owing to the introduction of a new distinguishable degree-of-freedom, even extremely weak signals can be discriminated and separated from a strong noise produced in SBS processes. The mechanism demonstrated in this proof-of-principle work provides a practical way for quasi-noise-free photonic-phononic operation, which is still valid in waveguides supporting multi-orthogonal spatial modes, permits more flexibility and robustness for future SBS devices.
Spin-flip relaxation via optical phonon scattering in quantum dots
Wang, Zi-Wu; Liu, Lei; Li, Shu-Shen
2013-12-14
Based on the spin-orbit coupling admixture mechanism, we theoretically investigate the spin-flip relaxation via optical phonon scattering in quantum dots by considering the effect of lattice relaxation due to the electron-acoustic phonon deformation potential coupling. The relaxation rate displays a cusp-like structure (or a spin hot spot) that becomes more clearly with increasing temperature. We also calculate the relaxation rate of the spin-conserving process, which follows a Gaussian form and is several orders of magnitude larger than that of spin-flip process. Moreover, we find that the relaxation rate displays the oscillatory behavior due to the interplay effects between the magnetic and spatial confinement for the spin-flip process not for the spin-conserving process. The trends of increasing and decreasing temperature dependence of the relaxation rates for two relaxation processes are obtained in the present model.