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Sample records for aerosol backscatter profiles

  1. Multi-wavelength profiles of aerosol backscatter over Lauder, New Zealand, 24 November 1992

    NASA Technical Reports Server (NTRS)

    Mckenzie, R. L.; Rosen, J. M.; Kjome, N. T.; Mcgee, T. J.; Gross, M. R.; Singh, U. N.; Ferrare, R. F.; Kimvilakani, P.; Uchino, O.; Nagai, T.

    1994-01-01

    Simultaneous profiles of aerosol backscatter ratio were measured over Lauder, New Zealand (45 deg S, 170 deg E) on the night of November 24, 1992. Instrumentation comprised two complementary lidar systems and a backscattersonde, to give measurements at wavelengths 351, 490, 532, and 940 nm. The data from the lidars and the backscattersonde were self-consistent, enabling the wavelength dependence of aerosol backscatter to be determined as a function of altitude. This wavelength-dependence is a useful parameter in radiative transfer calculations. In the stratosphere, the average wavelength exponent between 351 and 940 nm was -1.23 +/- 0.1, which was in good agreement with values derived from measured physical properties of aerosols.

  2. Aerosol backscatter studies supporting LAWS

    NASA Technical Reports Server (NTRS)

    Rothermel, Jeffry

    1989-01-01

    Optimized Royal Signals and Radar Establishment (RSRE), Laser True Airspeed System (LATAS) algorithm for low backscatter conditions was developed. The algorithm converts backscatter intensity measurements from focused continuous-wave (CW) airborne Doppler lidar into backscatter coefficients. The performance of optimized algorithm under marginal backscatter signal conditions was evaluated. The 10.6 micron CO2 aerosol backscatter climatologies were statistically analyzed. Climatologies reveal clean background aerosol mode near 10(exp -10)/kg/sq m/sr (mixing ratio units) through middle and upper troposhere, convective mode associated with planetary boundary layer convective activity, and stratospheric mode associated with volcanically-generated aerosols. Properties of clean background mode are critical to design and simulation studies of Laser Atmospheric Wind Sounder (LAWS), a MSFC facility Instrument on the Earth Observing System (Eos). Previous intercomparisons suggested correlation between aerosol backscatter at CO2 wavelength and water vapor. Field measurements of backscatter profiles with MSFC ground-based Doppler lidar system (GBDLS) were initiated in late FY-88 to coincide with independent program of local rawinsonde releases and overflights by Multi-spectral Atmospheric Mapping Sensor (MAMS), a multi-channel infrared radiometer capable of measuring horizontal and vertical moisture distributions. Design and performance simulation studies for LAWS would benefit from the existence of a relationship between backscatter and water vapor.

  3. CART and GSFC raman lidar measurements of atmospheric aerosol backscattering and extinction profiles for EOS validation and ARM radiation studies

    NASA Technical Reports Server (NTRS)

    Ferrare, R. A.; Turner, D. D.; Melfi, S. H.; Whiteman, D. N.; Schwenner, G.; Evans, K. D.; Goldsmith, J. E. M.; Tooman, T.

    1998-01-01

    The aerosol retrieval algorithms used by the Moderate-Resolution Imaging Spectroradiometer (MODIS) and Multi-Angle Imaging SpectroRadiometer (MISR) sensors on the Earth Observing Satellite (EOS) AM-1 platform operate by comparing measured radiances with tabulated radiances that have been computed for specific aerosol models. These aerosol models are based almost entirely on surface and/or column averaged measurements and so may not accurately represent the ambient aerosol properties. Therefore, to validate these EOS algorithms and to determine the effects of aerosols on the clear-sky radiative flux, we have begun to evaluate the vertical variability of ambient aerosol properties using the aerosol backscattering and extinction profiles measured by the Cloud and Radiation Testbed (CART) and NASA Goddard Space Flight Center (GSFC) Raman Lidars. Using the procedures developed for the GSFC Scanning Raman Lidar (SRL), we have developed and have begun to implement algorithms for the CART Raman Lidar to routinely provide profiles of aerosol extinction and backscattering during both nighttime and ,daytime operations. Aerosol backscattering and extinction profiles are computed for both lidar systems using data acquired during the 1996 and 1997 Water Vapor Intensive Operating Periods (IOPs). By integrating these aerosol extinction profiles, we derive measurements of aerosol optical thickness and compare these with coincident sun photometer measurements. We also use these measurements to measure the aerosol extinction/backscatter ratio S(sub a) (i.e. 'lidar ratio'). Furthermore, we use the simultaneous water vapor measurements acquired by these Raman lidars to investigate the effects of water vapor on aerosol optical properties.

  4. Analysis of DIAL/HSRL aerosol backscatter and extinction profiles during the SEAC4RS campaign with an aerosol assimilation system

    NASA Astrophysics Data System (ADS)

    Weaver, C. J.; da Silva, A. M., Jr.; Colarco, P. R.; Randles, C. A.

    2015-12-01

    We retrieve aerosol concentrations and optical information from vertical profiles of airborne 532 nm extinction and 532 and 1064 nm backscatter measurements made during the SEAC4RS summer 2013 campaign. The observations are from the High Spectral Resolution Lidar (HSRL) Airborne Differential Absorption Lidar (DIAL) on board the NASA DC-8. Instead of retrieving information about aerosol microphysical properties such as indexes of refraction, we seek information more directly applicable to an aerosol transport model - in our case the Goddard Chemistry Aerosol Radiation and Transport (GOCART) module used in the GEOS-5 Earth modeling system. A joint atmosphere/aerosol mini-reanalysis was performed for the SEAC4RS period using GEOS-5. The meteorological reanalysis followed the MERRA-2 atmospheric reanalysis protocol, and aerosol information from MODIS, MISR, and AERONET provided a constraint on the simulated aerosol optical depth (i.e., total column loading of aerosols). We focus on the simulated concentrations of 10 relevant aerosol species simulated by the GOCART module: dust, sulfate, and organic and black carbon. Our first retrieval algorithm starts with the SEAC4RS mini-reanalysis and adjusts the concentration of each GOCART aerosol species so that differences between the observed and simulated backscatter and extinction measurements are minimized. In this case, too often we are unable to simulate the observations by simple adjustment of the aerosol concentrations. A second retrieval approach adjusts both the aerosol concentrations and the optical parameters (i.e., assigned mass extinction efficiency) associated with each GOCART species. We present results from DC-8 flights over smoke from forest fires over the western US using both retrieval approaches. Finally, we compare our retrieved quantities with in-situ observations of aerosol absorption, scattering, and mass concentrations at flight altitude.

  5. Theory of CW lidar aerosol backscatter measurements and development of a 2.1 microns solid-state pulsed laser radar for aerosol backscatter profiling

    NASA Technical Reports Server (NTRS)

    Kavaya, Michael J.; Henderson, Sammy W.; Frehlich, R. G.

    1991-01-01

    The performance and calibration of a focused, continuous wave, coherent detection CO2 lidar operated for the measurement of atmospheric backscatter coefficient, B(m), was examined. This instrument functions by transmitting infrared (10 micron) light into the atmosphere and collecting the light which is scattered in the rearward direction. Two distinct modes of operation were considered. In volume mode, the scattered light energy from many aerosols is detected simultaneously, whereas in the single particle mode (SPM), the scattered light energy from a single aerosol is detected. The analysis considered possible sources of error for each of these two cases, and also considered the conditions where each technique would have superior performance. The analysis showed that, within reasonable assumptions, the value of B(m) could be accurately measured by either the VM or the SPM method. The understanding of the theory developed during the analysis was also applied to a pulsed CO2 lidar. Preliminary results of field testing of a solid state 2 micron lidar using a CW oscillator is included.

  6. Comparison of Aerosol Backscatter and Extinction Profiles Based on the Earlinet Database and the Single Calculus Chain for Thessaloniki Greece (2001-2014)

    NASA Astrophysics Data System (ADS)

    Voudouri, K.; Siomos, N.; Giannakaki, E.; Amiridis, V.; d'Amico, G.; Balis, D. S.

    2016-06-01

    Aerosol backscatter and extinction coefficient profiles derived by the Single Calculus Chain (SCC) algorithm, which was developed within the European Aerosol Research Lidar Network (EARLINET) are compared with profiles derived by the operational inversion algorithm of Thessaloniki. Measurements performed during the period 2001-2014, that have already been uploaded in the EARLINET database, are considered in this study. The objective of this study is to verify, for the case of Thessaloniki, the consistency of the climatology of the aerosol profiles based on SCC and the EARLINET database data respectively. In this paper we show example comparisons for each lidar product submitted in the official database.

  7. Lidar backscattering measurements of background stratospheric aerosols

    NASA Technical Reports Server (NTRS)

    Remsberg, E. E.; Northam, G. B.; Butler, C. F.

    1979-01-01

    A comparative lidar-dustsonde experiment was conducted in San Angelo, Texas, in May 1974 in order to estimate the uncertainties in stratospheric-aerosol backscatter for the NASA Langley 48-inch lidar system. The lidar calibration and data-analysis procedures are discussed. Results from the Texas experiment indicate random and systematic uncertainties of 35 and 63 percent, respectively, in backscatter from a background stratospheric-aerosol layer at 20 km.

  8. Aerosol backscatter lidar calibration and data interpretation

    NASA Technical Reports Server (NTRS)

    Kavaya, M. J.; Menzies, R. T.

    1984-01-01

    A treatment of the various factors involved in lidar data acquisition and analysis is presented. This treatment highlights sources of fundamental, systematic, modeling, and calibration errors that may affect the accurate interpretation and calibration of lidar aerosol backscatter data. The discussion primarily pertains to ground based, pulsed CO2 lidars that probe the troposphere and are calibrated using large, hard calibration targets. However, a large part of the analysis is relevant to other types of lidar systems such as lidars operating at other wavelengths; continuous wave (CW) lidars; lidars operating in other regions of the atmosphere; lidars measuring nonaerosol elastic or inelastic backscatter; airborne or Earth-orbiting lidar platforms; and lidars employing combinations of the above characteristics.

  9. SAGE II aerosol correlative observations - Profile measurements

    NASA Technical Reports Server (NTRS)

    Osborn, M. T.; Rosen, J. M.; Mccormick, M. P.; Wang, Pi-Huan; Livinfston, J. M.

    1989-01-01

    Profiles of the aerosol extinction measurements from the Stratospheric Aerosol and Gas Experiment (SAGE) II are compared with profiles from five correlative experiments between November 1984 and July 1986. The correlative profiles were derived from six-channel dustsonde measurements and two-wavelength lidar backscatter data. The correlation between the dustsonde- and lidar-derived measurements and the SAGE II data is good, validating the SAGE II lower stratospheric aerosol extinction measurements.

  10. Wavelength dependence of aerosol backscatter coefficients obtained by multiple wavelength Lidar measurements

    NASA Technical Reports Server (NTRS)

    Sasano, Y.; Browell, E. V.

    1986-01-01

    Aerosols are often classified into several general types according to their origins and composition, such as maritime, continental, and stratospheric aerosols, and these aerosol types generally have different characteristics in chemical and physical properties. The present study aims at demonstrating the potential for distinguishing these aerosol types by the wavelength dependence of their backscatter coefficients obtained from quantitative analyses of multiple wavelength lidar signals. Data from the NASA Airborne Differential Abosrption lidar (DIAL) S ystems, which can measure aerosol backscatter profiles at wavelenghts of 300, 600, and 1064 nm and ozone profiles of backscatter coefficients for these three wavelength were derived from the observations of aerosols of different types. Observations were performed over the Atlantic Ocean, the Southwestern United States, and French Guyana.

  11. Vertical Aerosol Backscatter Variability from an Airborne Focused Continuous Wave CO2 Lidar

    NASA Technical Reports Server (NTRS)

    Jarzembski, Maurice A.; Srivastava, Vandana; Rothermel, Jeffry

    1998-01-01

    Atmospheric aerosol backscatter measurements using a continuous wave focused Doppler lidar at 9.1 micron wavelength were obtained over western North America and the Pacific Ocean during 13 - 26 September, 1995 as part of National Aeronautics and Space Administration's (NASA) Multi-center Airborne Coherent Atmospheric Wind Sensor (MACAWS) mission on board the NASA DC8 aircraft. Backscatter variability was measured for approximately 52 flight hours, covering equivalent horizontal distance of approximately 25,000 km in the troposphere. Quasi-vertical backscatter profiles were also obtained during various ascents and descents which ranged between approximately 0.1 to 12.0 km altitude. Aerosol haze layers were encountered at different altitudes. Similarities and differences for aerosol loading over land and over ocean were observed. A mid-tropospheric aerosol backscatter background mode was found with modal value approximately 1O(exp -10)/m/sr, consistent with previous airborne and ground-based datasets.

  12. Analysis of lidar backscatter profiles in optically thin clouds.

    PubMed

    Young, S A

    1995-10-20

    The solution of the lidar equation for profiles of backscatter and extinction in optically thin clouds is constrained by values of the cloud transmittance determined from the elastically scattered lidar signals below and above the cloud. The method is extended to those cases in which an aerosol layer lies below or above the cloud layer. Examples are given in both cases. An analytical expression for the average lidar ratio in the cloud is derived for those cases in which molecular scattering is significant.

  13. Raman Lidar Measurements of the Aerosol Extinction-to-Backscatter Ratio Over the Southern Great Plains

    SciTech Connect

    Ferrare, Richard; Turner, David D.; Brasseur, L. H.; Feltz, W. F.; Dubovik, O.; Tooman, Tim P.

    2001-09-16

    We derive profiles of the aerosol extinction-to-backscatter ratio, Sa, at 355 nm using aerosol extinction and backscatter profiles measured during 1998 and 1999 by the operational Raman lidar at the Department of Energy Atmospheric Radiation Measurement program Southern Great Plains site in north central Oklahoma. Data from this Raman/Rayleigh-Mie lidar, which measures Raman scattering from nitrogen as well as the combined molecular (Rayleigh) and aerosol (Mie) scattering at the laser wavelength, are used to derive aerosol extinction and backscattering independently as a function of altitude. Because this lidar operates at 355 nm, where molecular backscattering is comparable with aerosol backscattering, Sa retrievals are generally limited to conditions where the aerosol extinction at 355 nm is > 0.03 km-1. The mean value of Sa at 355 nm derived for this period was 60 sr with a standard deviation of 12 sr. Sa was generally about 5-10 sr higher during high aerosol optical thickness (AOT) (> 0.3) conditions than during low AOT (< 0.1). A similar increase in Sa was found when the relative humidity increased from 30 to 80%. Large (> 15%) variations in the vertical profile of Sa occurred about 30% of the time, which implies significant variability in the vertical distribution of aerosol size distribution, shape, and/or composition often occurs. The Raman lidar measurements of Sa were compared with estimates of particle size and refractive index derived from an algorithm that uses ground-based Sun photometer measurements of Sun and sky radiance. For 17 cases of coincident Raman lidar and Sun and sky radiance measurements, Sa was linearly correlated with the aerosol fine mode effective radius and the volume ratio of fine/coarse particles.

  14. Raman lidar measurements of aerosol extinction and backscattering 1. Methods and comparisons

    SciTech Connect

    Ferrare, R.A.; Melfi, S.H.; Whiteman, D.N.; Evans, K.D.

    1998-08-01

    This paper examines the aerosol backscattering and extinction profiles measured at night by the NASA Goddard Space Flight Center Scanning Raman Lidar (SRL) during the remote cloud sensing (RCS) intensive operations period (IOP) at the Department of Energy Atmospheric Radiation Measurement (ARM) southern Great Plains (SGP) site in April 1994. These lidar data are used to derive aerosol profiles for altitudes between 0.015 and 5 km. Since this lidar detects Raman scattering from nitrogen and oxygen molecules as well as the elastic scattering from molecules and aerosols, it measures both aerosol backscattering and extinction simultaneously. The aerosol extinction/backscattering ratio varied between approximately 30 sr and 75 sr at 351 nm. Aerosol optical thicknesses derived by integrating the lidar profiles of aerosol extinction measured at night between 0.1 and 5 km are found to be about 10{endash}40{percent} lower than those measured by a Sun photometer during the day. This difference is attributed to the contribution by stratospheric aerosols not included in the lidar estimates as well as to diurnal differences in aerosol properties and concentrations. Aerosol profiles close to the surface were acquired by pointing the lidar nearly horizontally. Measurements of aerosol scattering from a tower-mounted nephelometer are found to be 40{percent} lower than lidar measurements of aerosol extinction over a wide range of relative humidities even after accounting for the difference in wavelengths. The reasons for this difference are not clear but may be due to the inability of the nephelometer to accurately measure scattering by large particles. {copyright} 1998 American Geophysical Union

  15. Raman Lidar Measurements of Aerosol Extinction and Backscattering. Report 1; Methods and Comparisons

    NASA Technical Reports Server (NTRS)

    Ferrare, R. A.; Melfi, S. H.; Whiteman, D. N.; Evans, K. D.; Leifer, R.

    1998-01-01

    This paper examines the aerosol backscattering and extinction profiles measured at night by the NASA Goddard Space Flight Center Scanning Raman Lidar (SRL) during the remote cloud sensing (RCS) intensive operations period (IOP) at the Department of Energy Atmospheric Radiation Measurement (ARM) southern Great Plains (SGP) site in April 1994. These lidar data are used to derive aerosol profiles for altitudes between 0.0 1 5 and 5 km. Since this lidar detects Raman scattering from nitrogen and oxygen molecules as well as the elastic scattering from molecules and aerosols, it measures both aerosol backscattering and extinction simultaneously. The aerosol extinction/backscattering ratio varied between approximately 30 sr and 75 sr at 351 nm. Aerosol optical thicknesses derived by integrating the lidar profiles of aerosol extinction measured at night between 0. I and 5 km are found to be about 10-40% lower than those measured by a Sun photometer during the day. This difference is attributed to the contribution by stratospheric aerosols not included in the lidar estimates as well as to diurnal differences in aerosol properties and concentrations. Aerosol profiles close to the surface were acquired by pointing the lidar nearly horizontally. Measurements of aerosol scattering from a tower-mounted nephelometer are found to be 40% lower than lidar measurements of aerosol extinction over a wide range of relative humidities even after accounting for the difference in wavelengths. The reasons for this difference are not clear but may be due to the inability of the nephelometer to accurately measure scattering by large particles.

  16. Comparison of temperature and humidity profiles with elastic-backscatter lidar data

    SciTech Connect

    Soriano, C. |; Buttler, W.T.; Baldasano, J.M.

    1995-04-01

    This contribution analyzes elastic-backscatter lidar data and temperature and humidity profiles from radiosondes acquired in Barcelona in July 1992. Elastic-backscatter lidar data reveal the distribution of aerosols within the volume of atmosphere scanned. By comparing this information with temperature and humidity profiles of the atmosphere at a similar time, we are able to asses de relationship among aerosol distribution and atmospheric stability or water content, respectively. Comparisons have shown how lidar`s revealed layers of aerosols correspond to atmospheric layers with different stability condition and water content.

  17. Aerosol Lidar for the Relative Backscatter Amplification Measurements

    NASA Astrophysics Data System (ADS)

    Razenkov, Igor A.; Banakh, Victor A.; Nadeev, Alexander I.

    2016-06-01

    Backscatter amplification presents only in a turbulent atmosphere, when the laser beam is propagates twice through the same inhomogeneities. We proposed technical solution to detect backscatter amplification. An aerosol micro pulse lidar with a beam expansion via receiving telescope was built to study this effect. Our system allows simultaneous detection of two returns from the same scattering volume: exactly on the axis of the laser beam and off the axis.

  18. Aerosol Backscatter and Extinction Retrieval from Airborne Coherent Doppler Wind Lidar Measurements

    NASA Astrophysics Data System (ADS)

    Chouza, F.; Reitebuch, O.; Groß, S.; Rahm, S.; Freudenthaler, V.; Toledano, C.; Weinzierl, B.

    2016-06-01

    A novel method for coherent Doppler wind lidars (DWLs) calibration is shown in this work. Concurrent measurements of a ground based aerosol lidar operating at 532 nm and an airborne DWL at 2 μm are used in combination with sun photometer measurements for the retrieval of backscatter and extinction profiles. The presented method was successfully applied to the measurements obtained during the Saharan Aerosol Long-range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE: http://www.pa.op.dlr.de/saltrace), which aimed to characterize the Saharan dust long range transport between Africa and the Caribbean.

  19. Vertical distribution of near-ground aerosol backscattering coefficient measured by a CCD side-scattering lidar

    NASA Astrophysics Data System (ADS)

    Tao, Zongming; Liu, Dong; Ma, Xiaomin; Shi, Bo; Shan, Huihui; Zhao, Ming; Xie, Chenbo; Wang, Yingjian

    2015-09-01

    The near-ground aerosols have the most impact on the human beings. Its fine spatial and temporal distribution, with which the environmental and meteorological departments concern themselves most, has not been elaborated very well due to the unavailable measurement tools. We present the continuous observations of the vertical profile of near-ground aerosol backscattering coefficients by employing our self-developed side-scattering lidar system based on charge-coupled device camera. During the experimental period from April 2013 to August 2014, four catalogs of aerosol backscattering coefficient profiles are found in the near ground. The continuous measurement is revealed by the contour plots measured during the whole night. These experimental results indicate that the aerosol backscattering coefficients in near ground are inhomogeneous and vary with altitude and time, which are very useful for the model researchers to study the regional air pollution and its climate impact.

  20. Comparison of Modeled Backscatter using Measured Aerosol Microphysics with Focused CW Lidar Data over Pacific

    NASA Technical Reports Server (NTRS)

    Srivastava, Vandana; Clarke, Antony D.; Jarzembski, Maurice A.; Rothermel, Jeffry

    1997-01-01

    During NASA's GLObal Backscatter Experiment (GLOBE) II flight mission over the Pacific Ocean in May-June 1990, extensive aerosol backscatter data sets from two continuous wave, focused CO2 Doppler lidars and an aerosol microphysics data set from a laser optical particle counter (LOPC) were obtained. Changes in aerosol loading in various air masses with associated changes in chemical composition, from sulfuric acid and sulfates to dustlike crustal material, significantly affected aerosol backscatter, causing variation of about 3 to 4 orders of magnitude. Some of the significant backscatter features encountered in different air masses were the low backscatter in subtropical air with even lower values in the tropics near the Intertropical Convergence Zone (ITCZ), highly variable backscatter in the ITCZ, mid-tropospheric aerosol backscatter background mode, and high backscatter in an Asian dust plume off the Japanese coast. Differences in aerosol composition and backscatter for northern and southern hemisphere also were observed. Using the LOPC measurements of physical and chemical aerosol properties, we determined the complex refractive index from three different aerosol mixture models to calculate backscatter. These values provided a well-defined envelope of modeled backscatter for various atmospheric conditions, giving good agreement with the lidar data over a horizontal sampling of approximately 18000 km in the mid-troposphere.

  1. Characteristics of CALIOP attenuated backscatter noise: implication for cloud/aerosol detection

    NASA Astrophysics Data System (ADS)

    Wu, D. L.; Chae, J. H.; Lambert, A.; Zhang, F. F.

    2011-03-01

    A research algorithm is developed for noise evaluation and feature detection of the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) Level 1 (L1) backscatter data with an emphasis on cloud/aerosol features in the upper troposphere and lower stratosphere (UT/LS). CALIOP measurement noise of the version v2.01 and v2.02 L1 backscatter data aggregated to (5 km) horizontal resolution is analyzed with two approaches in this study. One is to compare the observed and modeled molecular scatter profiles by scaling the modeled profile (with a fitted scaling factor α) to the observed clear-sky backscatter profiles. This scaling α value is sensitive to errors in the calibrated backscatter and the atmospheric model used. Most of the nighttime 532-nm α values are close to unity, as expected, but an abrupt drop occurred in October 2008 in the daytime 532-nm α, which is likely indicative of a problem in the v2.02 daytime calibrated data. The 1064-nm night α is generally close to 2 while its day α is ~3. The other approach to evaluate the lidar measurement noise is to use the calibrated lidar backscatter data at altitudes above 19 km. With this method, the 532-nm and 1064-nm measurement noises are analyzed and characterized individually for each profile in terms of the mean (μ) and standard deviation (σ), showing larger σ values in general over landmasses or bright surfaces during day and in radiation-hard regions during night. A significant increasing trend is evident in the nighttime 1064-nm σ, which is likely responsible for the increasing difference between the feature occurrence frequencies (532-nm vs. 1064-nm) derived from this study. For feature detection with the research algorithm, we apply a σ-based method to the aggregated L1 data. The derived morphology of feature occurrence frequency is in general agreement with that obtained from the Level 2 (L2) 05 km_CLAY+05 km_ALAY products at 5 km horizontal resolution. Finally, a normalized probability density

  2. Multiwavelength Comparison of Modeled and Measured Remote Tropospheric Aerosol Backscatter Over Pacific Ocean

    NASA Technical Reports Server (NTRS)

    Cutten, D. R.; Pueschel, R. F.; Srivastava, V.; Clarke, A. D.; Rothermel, J.; Spinhirne, J. D.; Menzies, R. T.

    1996-01-01

    Aerosol concentrations and size distributions in the middle and upper troposphere over the remote Pacific Ocean were measured with a forward scattering spectrometer probe (FSSP) on the NASA DC-8 aircraft during NASA's Global Backscatter Experiment (GLOBE) in May-June 1990. The FSSP size channels were recalibrated based on refractive index estimates from flight-level aerosol volatility measurements with a collocated laser optical particle counter (LOPC). The recalibrated FSSP size distributions were averaged over 100-s intervals, fitted with lo-normal distributions and used to calculate aerosol backscatter coefficients at selected wavelengths. The FSSP-derived backscatter estimates were averaged over 300-s intervals to reduce large random fluctuations. The smoothed FSSP aerosol backscatter coefficients were then compared with LOPC-derived backscatter values and with backscatter measured at or near flight level from four lidar systems operating at 0.53, 1.06, 9.11, 9.25, and 10.59 micrometers. Agreement between FSSP-derived and lidar-measured backscatter was generally best at flight level in homogeneous aerosol fields and at high backscatter values. FSSP data often underestimated low backscatter values especially at the longer wavelengths due to poor counting statistics for larger particles (greater than 0.8 micrometers diameter) that usually dominate aerosol backscatter at these wavelengths. FSSP data also underestimated backscatter at shorter wavelengths when particles smaller than the FSSP lower cutoff diameter (0.35 micrometers) made significant contributions to the total backscatter.

  3. Retrieval of stratospheric aerosol size distributions and integral properties from simulated lidar backscatter measurements.

    PubMed

    Yue, G K

    2000-10-20

    A new approach for retrieving aerosol properties from extinction spectra is extended to retrieve aerosol properties from lidar backscatter measurements. In this method it is assumed that aerosol properties are expressed as a linear combination of backscatters at three or fewer wavelengths commonly used in lidar measurements. The coefficients in the weighted linear combination are obtained by minimization of the retrieval error averaged for a set of testing size distributions. The formulas can be used easily by investigators to retrieve aerosol properties from lidar backscatter measurements such as the Lidar In-Space Technology Experiment and Pathfinder Instruments for Clouds and Aerosols Spaceborne Observations.

  4. Aerosol size distribution, composition, and CO2 backscatter

    NASA Astrophysics Data System (ADS)

    Clarke, Antony D.; Porter, John N.

    1991-03-01

    The aerosol size distribution, composition, and CO2 backscatter at 10.6 microns (beta-CO2) were measured continuosly at the Mauna Loa Observatory (Hawaii) during January-March and November-December, 1988 periods to compare the characteristics of periods associated with appreciable Asian dust transport to that site (January-March) with those of periods characterized by low-dust condition. The aerosol size distribution in the range 0.15 micron to 7.6 microns was measured at temperatures of 40, 150, and 340 C to differentiate between volatile and nonvolatile aerosols. Large ranges of variability was found in measurements of aerosol size distribution during both periods, but the average distributions were similar for both the high-dust and the low-dust periods. However, values for beta-CO2 were more elevated (by about six times) during periods associated with active Asian dust transport to the observatory site than during the low-dust periods.

  5. Potential of lidar backscatter data to estimate solar aerosol radiative forcing

    NASA Astrophysics Data System (ADS)

    Wendisch, Manfred; Müller, Detlef; Mattis, Ina; Ansmann, Albert

    2006-02-01

    The potential to estimate solar aerosol radiative forcing (SARF) in cloudless conditions from backscatter data measured by widespread standard lidar has been investigated. For this purpose 132 days of sophisticated ground-based Raman lidar observations (profiles of particle extinction and backscatter coefficients at 532 nm wavelength) collected during two campaigns [the European Aerosol Research Lidar Network (EARLINET) and the Indian Ocean Experiment (INDOEX)] were analyzed. Particle extinction profiles were used as input for radiative transfer simulations with which to calculate the SARF, which then was plotted as a function of the column (i.e., height-integrated) particle backscatter coefficient (betac). A close correlation between the SARF and betac was found. SARF-betac parameterizations in the form of polynomial fits were derived that exhibit an estimated uncertainty of +/-(10-30)%. These parameterizations can be utilized to analyze data of upcoming lidar satellite missions and for other purposes. The EARLINET-based parameterizations can be applied to lidar measurements at mostly continental, highly industrialized sites with limited maritime influence (Europe, North America), whereas the INDOEX parameterizations rather can be employed in polluted maritime locations, e.g., coastal regions of south and east Asia.

  6. Potential of lidar backscatter data to estimate solar aerosol radiative forcing.

    PubMed

    Wendisch, Manfred; Müller, Detlef; Mattis, Ina; Ansmann, Albert

    2006-02-01

    The potential to estimate solar aerosol radiative forcing (SARF) in cloudless conditions from backscatter data measured by widespread standard lidar has been investigated. For this purpose 132 days of sophisticated ground-based Raman lidar observations (profiles of particle extinction and backscatter coefficients at 532 nm wavelength) collected during two campaigns [the European Aerosol Research Lidar Network (EARLINET) and the Indian Ocean Experiment (INDOEX)] were analyzed. Particle extinction profiles were used as input for radiative transfer simulations with which to calculate the SARF, which then was plotted as a function of the column (i.e., height-integrated) particle backscatter coefficient (beta(c)). A close correlation between the SARF and beta(c) was found. SARF-beta(c) parameterizations in the form of polynomial fits were derived that exhibit an estimated uncertainty of +/-(10-30)%. These parameterizations can be utilized to analyze data of upcoming lidar satellite missions and for other purposes. The EARLINET-based parameterizations can be applied to lidar measurements at mostly continental, highly industrialized sites with limited maritime influence (Europe, North America), whereas the INDOEX parameterizations rather can be employed in polluted maritime locations, e.g., coastal regions of south and east Asia.

  7. Ozone and Aerosol Retrieval from Backscattered Ultraviolet Radiation

    NASA Technical Reports Server (NTRS)

    Bhartia, Pawan K.

    2004-01-01

    In this presentation we will discuss the techniques to estimate total column ozone and aerosol absorption optical depth from the measurements of backscattered ultraviolet (buv) radiation. The total ozone algorithm has been used to create a unique record of the ozone layer, spanning more than 3 decades, from a series of instruments (BUV, SBUV, TOMS, SBUV/2) flown on NASA, NOAA, Japanese and Russian satellites. We will discuss how this algorithm can be considered a generalization of the well-known Dobson/Brewer technique that has been used to process data from ground-based instruments for many decades, and how it differs from the DOAS techniques that have been used to estimate vertical column densities of a host of trace gases from data collected by GOME and SCIAMACHY instruments. The BUV aerosol algorithm is most suitable for the detection of UV absorbing aerosols (smoke, desert dust, volcanic ash) and is the only technique that can detect aerosols embedded in clouds. This algorithm has been used to create a quarter century record of aerosol absorption optical depth using the BUV data collected by a series of TOMS instruments. We will also discuss how the data from the OM1 instrument launched on July 15,2004 will be combined with data from MODIS and CALIPSO lidar data to enhance the accuracy and information content of satellite-derived aerosol measurements. The OM1 and MODIS instruments are currently flying on EOS Aura and EOS Aqua satellites respectively, part of a constellation of satellites called the "A-train". The CALIPSO satellite is expected to join this constellation in mid 2005.

  8. Comparisons of Airborne HSRL and Modeled Aerosol Profiles

    NASA Astrophysics Data System (ADS)

    Ferrare, R. A.; Burton, S. P.; Hostetler, C. A.; Hair, J. W.; Ismail, S.; Rogers, R. R.; Notari, A.; Berkoff, T.; Butler, C. F.; Collins, J. E., Jr.; Fenn, M. A.; Scarino, A. J.; Clayton, M.; Mueller, D.; Chemyakin, E.; Fast, J. D.; Berg, L. K.; Randles, C. A.; Colarco, P. R.; daSilva, A.

    2014-12-01

    Aerosol profiles derived from a regional and a global model are compared with aerosol profiles acquired by NASA Langley Research Center (LaRC) airborne High Spectral Resolution Lidars (HSRLs) during recent field missions. We compare simulated aerosol profiles obtained from the WRF-Chem regional model with those measured by the airborne HSRL-2 instrument over the Atlantic Ocean east of Cape Cod in July 2012 during the Department of Energy Two-Column Aerosol Project (TCAP). While deployed on the LaRC King Air during TCAP, HSRL-2 acquired profiles of aerosol extinction at 355 and 532 nm, as well as aerosol backscatter and depolarization at 355, 532, and 1064 nm. Additional HSRL-2 data products include profiles of aerosol type, mixed layer depth, and aerosol microphysical parameters (e.g. effective radius, concentration). The HSRL-2 and WRF-Chem aerosol profiles are compared along the aircraft flight tracks. HSRL-2 profiles acquired during the NASA Deriving Information on Surface Conditions from COlumn and VERtically Resolved Observations Relevant to Air Quality (DISCOVER-AQ) mission over Houston during September 2013 are compared with the NASA Goddard Earth Observing System global model, version 5 (GEOS-5) profiles. In addition to comparing backscatter and extinction profiles, the fraction of aerosol extinction and optical thickness from various aerosol species from GEOS-5 are compared with aerosol extinction and optical thickness contributed by aerosol types derived from HSRL-2 data. We also compare aerosol profiles modeled by GEOS-5 with those measured by the airborne LaRC DIAL/HSRL instrument during August and September 2013 when it was deployed on the NASA DC-8 for the Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) mission. DIAL/HSRL measured extinction (532 nm), backscatter (532 and 1064 nm), and depolarization profiles (532 and 1064 nm) in both nadir and zenith directions during long transects over the

  9. Aerosol profiling by calibrated ceilometer data

    NASA Astrophysics Data System (ADS)

    Geiß, Alexander; Wiegner, Matthias

    2015-04-01

    Recently, networks of automated single-wavelength backscatter lidars ("ceilometers") were implemented, primarily by weather services. As a consequence, the potential of ceilometers to quantitatively determine the spatiotemporal distribution of atmospheric aerosols was investigated, to derive mixing layer heights for air quality studies and to assess optical properties. The main issues are the limited signal-to-noise ratio and the inherent problems of the calibration. We have studied several approaches for calibrating ceilometers, based on different numerical solutions and on auxiliary data of different remote sensing techniques. As a result, the backscatter coefficient can be determined with a relative accuracy of typically 10% and a time resolution in the order of 5 minutes. This parameter is used to estimate the mixing layer height by applying different techniques of averaging and pattern recognition. In this context, it is assumed that aerosols are a good tracer for the thermodynamic stratification of the troposphere. Our algorithm is fully automated and was tested for several commercially available ceilometers. For this purpose, a simplified version for non-calibrated ceilometers, based on the so called range corrected signal, was additionally developed. We used data of the CHM15k-x ceilometer (manufactured by Jenoptik) from more than 5 years of continuous operation by the LMU-MIM in Munich (Germany) to establish climatologies of mixing layer heights (MLH), cloud cover, cloud heights and vertical profiles of the backscatter coefficient. Among others, the mean diurnal cycle and the interannual variability of the MLH for different months were determined. Ceilometer derived MLH were also used to validate different parameterization of chemistry transport models and to validate forecasts of the dispersion of aerosol layers. For the latter applications backscatter coefficients are required. That means, a calibration of the ceilometers is mandatory.

  10. Recommendations for processing atmospheric attenuated backscatter profiles from Vaisala CL31 ceilometers

    NASA Astrophysics Data System (ADS)

    Kotthaus, Simone; O'Connor, Ewan; Münkel, Christoph; Charlton-Perez, Cristina; Haeffelin, Martial; Gabey, Andrew M.; Grimmond, C. Sue B.

    2016-08-01

    Ceilometer lidars are used for cloud base height detection, to probe aerosol layers in the atmosphere (e.g. detection of elevated layers of Saharan dust or volcanic ash), and to examine boundary layer dynamics. Sensor optics and acquisition algorithms can strongly influence the observed attenuated backscatter profiles; therefore, physical interpretation of the profiles requires careful application of corrections. This study addresses the widely deployed Vaisala CL31 ceilometer. Attenuated backscatter profiles are studied to evaluate the impact of both the hardware generation and firmware version. In response to this work and discussion within the CL31/TOPROF user community (TOPROF, European COST Action aiming to harmonise ground-based remote sensing networks across Europe), Vaisala released new firmware (versions 1.72 and 2.03) for the CL31 sensors. These firmware versions are tested against previous versions, showing that several artificial features introduced by the data processing have been removed. Hence, it is recommended to use this recent firmware for analysing attenuated backscatter profiles. To allow for consistent processing of historic data, correction procedures have been developed that account for artefacts detected in data collected with older firmware. Furthermore, a procedure is proposed to determine and account for the instrument-related background signal from electronic and optical components. This is necessary for using attenuated backscatter observations from any CL31 ceilometer. Recommendations are made for the processing of attenuated backscatter observed with Vaisala CL31 sensors, including the estimation of noise which is not provided in the standard CL31 output. After taking these aspects into account, attenuated backscatter profiles from Vaisala CL31 ceilometers are considered capable of providing valuable information for a range of applications including atmospheric boundary layer studies, detection of elevated aerosol layers, and model

  11. Characteristics of CALIOP attenuated backscatter noise: implication for cloud/aerosol detection

    NASA Astrophysics Data System (ADS)

    Wu, D. L.; Chae, J. H.; Lambert, A.; Zhang, F. F.

    2010-07-01

    To study cloud/aerosol features in the upper troposphere and lower stratosphere (UT/LS) with the NASA's A-Train sensors, a research algorithm is developed for a re-gridded CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) Level 1 (L1) backscatter dataset. This paper provides a detailed analysis of the measurement noise of this re-gridded dataset in order to compare the lidar measurements with other collocated measurements (e.g., CloudSat, Microwave Limb Sounder). The re-gridded dataset has a manageable data volume for multi-year analysis. It has a fixed (5 km) horizontal resolution, and the measurement error is derived empirically from the background-corrected backscatter profile on a profile-by-profile basis. The 532-nm and 1064-nm measurement noises, determined from the data at altitudes above 19 km, are analyzed and characterized in terms of the mean (μ), standard deviation (σ), and normalized probability density function (PDF). These noises show a larger variance over landmasses and bright surfaces during day, and in regions with enhanced flux of energetic particles during night, where the instrument's ability for feature detection is slightly degraded. An increasing trend in the nighttime 1064-nm σ appears to be significant, which likely causes the increasing differences in cloud occurrence frequency between the 532-nm and 1064-nm channels. Most of the CALIOP backscatter noise distributions exhibit a Gaussian-like behavior but the nighttime 532-nm perpendicular measurements show multi-Gaussian characteristics. We apply σ - based thresholds to detect cloud/aerosol features in the UT/LS from the subset L1 data. The observed morphology is similar to that from the Level 2 (L2) 05km_CLAY+05km_ALAY product, but the occurrence frequency obtained in this study is slightly lower than the L2 product due to differences in spatial averaging and detection threshold. In the case where the measurement noises of two data sets are different, the normalized PDF has

  12. Atmospheric aerosol and molecular backscatter imaging effects on direct detection LADAR

    NASA Astrophysics Data System (ADS)

    Youmans, Douglas G.

    2015-05-01

    Backscatter from atmospheric aerosols and molecular nitrogen and oxygen causes "clutter" noise in direct detection ladar applications operating within the atmosphere. The backscatter clutter is more pronounced in multiple pulse, high PRF ladars where pulse-averaging is used to increase operating range. As more and more pulses are added to the wavetrain the backscatter increases. We analyze the imaging of a transmitted Gaussian laser-mode multi-pulse wave-train scatteried off of aerosols and molecules at the focal plane including angular-slew rate resulting from optical tracking, angular lead-angle, and bistatic-optics spatial separation. The defocused backscatter images, from those pulses closest to the receiver, are analyzed using a simple geometrical optics approximation. Methods for estimating the aerosol number density versus altitude and the volume backscatter coefficient of the aerosols are also discussed.

  13. First results from the aerosol lidar and backscatter sonde intercomparison campaign STRAIT'1997 at table mountain facility during February-March 1997

    NASA Technical Reports Server (NTRS)

    Beyerle, G.; Gross, M. R.; Haner, D. A.; Kjome, N. T.; McDermid, I. S.; McGee, T. J.; Rosen, J. M.; Schaefer, H. - J.; Schrems, O.

    1998-01-01

    First results of an intercomparison measurement campaign between three aerosol lidar instruments and in-situ backscatter sondes performed at Table Mountain Facility (34.4 deg N, 117.7 deg E, 2280 m asl) in February-March 1997 are presented. During the campaign a total of 414 hours of lidar data were acquired by the Aerosol-Temperature-Lidar (ATL, Goddard Space Flight Center) the Mobile-aerosol-Raman-Lidar (MARL, Alfred Wegener Institute), and the TMF-Aerosol-Lidar (TAL, Jet Propulsion Laboratory), and four backscatter sondes were launched. From the data set altitude profiles of backscatter ratio and volume depolarization of stratospheric background aerosols at altitudes between 15 and 25 km and optically thin high-altitude cirrus clouds at altitudes below 13 km are derived. On the basis of a sulfuric acid aerosol model color ratio profiles obtained from two wavelength lidar data are compared to the corresponding profiles derived from the sonde observations. We find an excellent agreement between the in-situ and ATL lidar data with respect to backscatter and color ratio. Cirrus clouds were present on 16 of 26 nights during the campaign. Lidar observations with 17 minute temporal and 120-300 m spatial resolution indicate high spatial and temporal variability of the cirrus layers. Qualitative agreement is found between concurrent lidar measurements of backscatter ratio and volume depolarization.

  14. Remote Sensing of Aerosol Backscatter and Earth Surface Targets By Use of An Airborne Focused Continuous Wave CO2 Doppler Lidar Over Western North America

    NASA Technical Reports Server (NTRS)

    Jarzembski, Maurice A.; Srivastava, Vandana; Goodman, H. Michael (Technical Monitor)

    2000-01-01

    Airborne lidar systems are used to determine wind velocity and to measure aerosol or cloud backscatter variability. Atmospheric aerosols, being affected by local and regional sources, show tremendous variability. Continuous wave (cw) lidar can obtain detailed aerosol loading with unprecedented high resolution (3 sec) and sensitivity (1 mg/cubic meter) as was done during the 1995 NASA Multi-center Airborne Coherent Atmospheric Wind Sensor (MACAWS) mission over western North America and the Pacific Ocean. Backscatter variability was measured at a 9.1 micron wavelength cw focused CO2 Doppler lidar for approximately 52 flight hours, covering an equivalent horizontal distance of approximately 30,000 km in the troposphere. Some quasi-vertical backscatter profiles were also obtained during various ascents and descents at altitudes that ranged from approximately 0.1 to 12 km. Similarities and differences for aerosol loading over land and ocean were observed. Mid-tropospheric aerosol backscatter background mode was approximately 6 x 10(exp -11)/ms/r, consistent with previous lidar datasets. While these atmospheric measurements were made, the lidar also retrieved a distinct backscatter signal from the Earth's surface from the unfocused part of the focused cw lidar beam during aircraft rolls. Atmospheric backscatter can be highly variable both spatially and temporally, whereas, Earth-surface backscatter is relatively much less variant and can be quite predictable. Therefore, routine atmospheric backscatter measurements by an airborne lidar also give Earth surface backscatter which can allow for investigating the Earth terrain. In the case where the Earth's surface backscatter is coming from a well-known and fairly uniform region, then it can potentially offer lidar calibration opportunities during flight. These Earth surface measurements over varying Californian terrain during the mission were compared with laboratory backscatter measurements using the same lidar of various

  15. [Obtaining aerosol backscattering coefficient using pure rotational Raman-Mie scattering spectrum].

    PubMed

    Rong, Wei; Chen, Si-Ying; Zhang, Yin-Chao; Chen, He; Guo, Pan

    2012-11-01

    Both the traditional Klett and Fernald methods used to obtain atmospheric aerosol backscattering coefficient require the hypothesis of relationship between the extinction coefficient and backscattering coefficient, and this will bring error. According to the theory that the pure rotational Raman backscattering coefficient is only related to atmospheric temperature and pressure, a new method is presented for inverting aerosol backscattering coefficient, which needed the intensity of elastic scattering and rotational Raman combined with atmospheric temperature and pressure obtained with the sounding balloons in this article. This method can not only eliminate the errors of the traditional Klett and Fernald methods caused by the hypothesis, but also avoid the error caused by the correction of the overlap. Finally, the aerosol backscattering coefficient was acquired by using this method and the data obtained via the Raman-Mie scattering Lidar of our lab. And the result was compared with that of Klett and Fernald. PMID:23387171

  16. Vertical variability of aerosol backscatter from an airborne-focused continuous-wave CO2 lidar at 9.1-microm wavelength.

    PubMed

    Jarzembski, M A; Srivastava, V; Rothermel, J

    1999-02-20

    Atmospheric aerosol backscatter measurements taken with a continuous-wave focused Doppler lidar at 9.1-microm wavelength were obtained over western North America and the Pacific Ocean from 13 to 26 September 1995 as part of a NASA airborne mission. Backscatter variability was measured for approximately 52 flight hours, covering an equivalent horizontal distance of approximately 30,000 km in the troposphere. Some quasi-vertical backscatter profiles were also obtained during various ascents and descents at altitudes that ranged from approximately 0.1 to 12 km. Similarities and differences for aerosol loading over land and ocean were observed. A midtropospheric aerosol backscatter background mode near 3 x 10(-11) to 1 x 10(-10) m(-1) sr(-1) was obtained, which is consistent with those of previous airborne and ground-based data sets. PMID:18305690

  17. Independent measurement of extinction and backscatter profiles in cirrus clouds by using a combined Raman elastic-backscatter lidar.

    PubMed

    Ansmann, A; Wandinger, U; Riebesell, M; Weitkamp, C; Michaelis, W

    1992-11-20

    Height profiles of the extinction and the backscatter coefficients in cirrus clouds are determined independently from elastic- and inelastic- (Raman) backscatter signals. An extended error analysis is given. Examples covering the measured range of extinction-to-backscatter ratios (lidar ratios) in ice clouds are presented. Lidar ratios between 5 and 15 sr are usually found. A strong variation between 2 and 20 sr can be observed within one cloud profile. Particle extinction coefficients determined from inelastic-backscatter signals and from elastic-backscatter signals by using the Klett method are compared. The Klett solution of the extinction profile can be highly erroneous if the lidar ratio varies along the measuring range. On the other hand, simple backscatter lidars can provide reliable information about the cloud optical depth and the mean cloud lidar ratio.

  18. On the Feasibility of Studying Shortwave Aerosol Radiative Forcing of Climate Using Dual-Wavelength Aerosol Backscatter Lidar

    NASA Technical Reports Server (NTRS)

    Redemann, Jens; Russell, Philip B.; Winker, David M.; McCormick, M. Patrick; Hipskind, R. Stephen (Technical Monitor)

    2000-01-01

    The current low confidence in the estimates of aerosol-induced perturbations of Earth's radiation balance is caused by the highly non-uniform compositional, spatial and temporal distributions of tropospheric aerosols on a global scale owing to their heterogeneous sources and short lifetimes. Nevertheless, recent studies have shown that the inclusion of aerosol effects in climate model calculations can improve agreement with observed spatial and temporal temperature distributions. In light of the short lifetimes of aerosols, determination of their global distribution with space-borne sensors seems to be a necessary approach. Until recently, satellite measurements of tropospheric aerosols have been approximate and did not provide the full set of information required to determine their radiative effects. With the advent of active aerosol remote sensing from space (e.g., PICASSO-CENA), the applicability fo lidar-derived aerosol 180 deg -backscatter data to radiative flux calculations and hence studies of aerosol effects on climate needs to be investigated.

  19. Intercomparison of aerosol extinction profiles retrieved from MAX-DOAS measurements

    NASA Astrophysics Data System (ADS)

    Frieß, U.; Klein Baltink, H.; Beirle, S.; Clémer, K.; Hendrick, F.; Henzing, B.; Irie, H.; de Leeuw, G.; Li, A.; Moerman, M. M.; van Roozendael, M.; Shaiganfar, R.; Wagner, T.; Wang, Y.; Xie, P.; Yilmaz, S.; Zieger, P.

    2016-07-01

    A first direct intercomparison of aerosol vertical profiles from Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations, performed during the Cabauw Intercomparison Campaign of Nitrogen Dioxide measuring Instruments (CINDI) in summer 2009, is presented. Five out of 14 participants of the CINDI campaign reported aerosol extinction profiles and aerosol optical thickness (AOT) as deduced from observations of differential slant column densities of the oxygen collision complex (O4) at different elevation angles. Aerosol extinction vertical profiles and AOT are compared to backscatter profiles from a ceilometer instrument and to sun photometer measurements, respectively. Furthermore, the near-surface aerosol extinction coefficient is compared to in situ measurements of a humidity-controlled nephelometer and dry aerosol absorption measurements. The participants of this intercomparison exercise use different approaches for the retrieval of aerosol information, including the retrieval of the full vertical profile using optimal estimation and a parametrised approach with a prescribed profile shape. Despite these large conceptual differences, and also differences in the wavelength of the observed O4 absorption band, good agreement in terms of the vertical structure of aerosols within the boundary layer is achieved between the aerosol extinction profiles retrieved by the different groups and the backscatter profiles observed by the ceilometer instrument. AOTs from MAX-DOAS and sun photometer show a good correlation (R>0.8), but all participants systematically underestimate the AOT. Substantial differences between the near-surface aerosol extinction from MAX-DOAS and from the humidified nephelometer remain largely unresolved.

  20. Transmitted beam profiles, integrated backscatter, and rangeresolved backscatter in inhomogeneous laboratory water droplet clouds.

    PubMed

    Bissonnette, L R; Smith, R B; Ulitsky, A; Houston, J D; Carswell, A I

    1988-06-15

    Using laser sources at wavelengths of 1.06 and 10.6 microm, transmitted beam profiles, integrated backscatter, and range-resolved backscatter were measured in laboratory-generated water droplet clouds. Clouds with carefully controlled properties were produced in a specially designed cloud chamber. Inhomogeneities were introduced by partitioning the cloud chamber into three adjacent sections separated by air screens. The measurements show the influence of multiple-scattering effects in both the forward and backward measurement geometries, and these are investigated as functions of optical depth, cloud inhomogeneity, and receiver field of view. These data are unique in many ways, and they provide a great deal of insight to the scattering processes which directly affect lidar-type measurements. As well, these measurements provide a welldocumented and detailed database for model validation. Very good agreement is demonstrated with the solutions derived from the multiscattering propagation model described in a companion paper [Appl. Opt. 27, 2478 (1988), same issue].

  1. Selection Algorithm for the CALIPSO Lidar Aerosol Extinction-to-Backscatter Ratio

    NASA Technical Reports Server (NTRS)

    Omar, Ali H.; Winker, David M.; Vaughan, Mark A.

    2006-01-01

    The extinction-to-backscatter ratio (S(sub a)) is an important parameter used in the determination of the aerosol extinction and subsequently the optical depth from lidar backscatter measurements. We outline the algorithm used to determine Sa for the Cloud and Aerosol Lidar and Infrared Pathfinder Spaceborne Observations (CALIPSO) lidar. S(sub a) for the CALIPSO lidar will either be selected from a look-up table or calculated using the lidar measurements depending on the characteristics of aerosol layer. Whenever suitable lofted layers are encountered, S(sub a) is computed directly from the integrated backscatter and transmittance. In all other cases, the CALIPSO observables: the depolarization ratio, delta, the layer integrated attenuated backscatter, beta, and the mean layer total attenuated color ratio, gamma, together with the surface type, are used to aid in aerosol typing. Once the type is identified, a look-up-table developed primarily from worldwide observations, is used to determine the S(sub a) value. The CALIPSO aerosol models include desert dust, biomass burning, background, polluted continental, polluted dust, and marine aerosols.

  2. Improving the detection of wind fields from LIDAR aerosol backscatter using feature extraction

    NASA Astrophysics Data System (ADS)

    Bickel, Brady R.; Rotthoff, Eric R.; Walters, Gage S.; Kane, Timothy J.; Mayor, Shane D.

    2016-04-01

    The tracking of winds and atmospheric features has many applications, from predicting and analyzing weather patterns in the upper and lower atmosphere to monitoring air movement from pig and chicken farms. Doppler LIDAR systems exist to quantify the underlying wind speeds, but cost of these systems can sometimes be relatively high, and processing limitations exist. The alternative is using an incoherent LIDAR system to analyze aerosol backscatter. Improving the detection and analysis of wind information from aerosol backscatter LIDAR systems will allow for the adoption of these relatively low cost instruments in environments where the size, complexity, and cost of other options are prohibitive. Using data from a simple aerosol backscatter LIDAR system, we attempt to extend the processing capabilities by calculating wind vectors through image correlation techniques to improve the detection of wind features.

  3. Particle backscatter and extinction profiling with the spaceborne high-spectral-resolution Doppler lidar ALADIN: methodology and simulations.

    PubMed

    Ansmann, Albert; Wandinger, Ulla; Le Rille, Olivier; Lajas, Dulce; Straume, Anne Grete

    2007-09-10

    The European Space Agency will launch the Atmospheric Laser Doppler Instrument (ALADIN) for global wind profile observations in the near future. The potential of ALADIN to measure the optical properties of aerosol and cirrus, as well, is investigated based on simulations. A comprehensive data analysis scheme is developed that includes (a) the correction of Doppler-shifted particle backscatter interference in the molecular backscatter channels (cross-talk effect), (b) a procedure that allows us to check the quality of the cross-talk correction, and (c) the procedures for the independent retrieval of profiles of the volume extinction and backscatter coefficients of particles considering the height-dependent ALADIN signal resolution. The error analysis shows that the particle backscatter and extinction coefficients, and the corresponding extinction-to-backscatter ratio (lidar ratio), can be obtained with an overall (systematic+statistical) error of 10%-15%, 15%-30%, and 20%-35%, respectively, in tropospheric aerosol and dust layers with extinction values from 50 to 200 Mm(-1); 700-shot averaging (50 km horizontal resolution) is required. Vertical signal resolution is 500 m in the lower troposphere and 1000 m in the free troposphere. In cirrus characterized by extinction coefficients of 200 Mm(-1) and an optical depth of >0.2, backscatter coefficients, optical depth, and column lidar ratios can be obtained with 25%-35% relative uncertainty and a horizontal resolution of 10 km (140 shots). In the stratosphere, only the backscatter coefficient of aerosol layers and polar stratospheric clouds can be retrieved with an acceptable uncertainty of 15%-30%. Vertical resolution is 2000 m.

  4. Backscatter measurements of aerosolized CB simulants with a frequency agile CO2 lidar

    NASA Astrophysics Data System (ADS)

    Vanderbeek, Richard; Gurton, Kristan

    2004-02-01

    A novel windowless chamber was developed to allow aerosol backscatter measurements with a frequency-agile CO2 lidar. The chamber utilizes curtains of air to contain the cloud, thus preventing the inevitable backscatter off of conventional windows from corrupting the desired measurements. This feature is critical because the CO2 lidar has a long (1 μs) pulse and the backscatter off the window cannot be temporally separated from the backscatter off the aerosol in the chamber. The chamber was designed for testing with a variety of CB simulants and interferents in both vapor and aerosol form and has been successfully shown to contain a cloud of known size, concentration, and particle size distribution for 10-15 minutes. This paper shows the results using Arizona road dust that was screened by the manufacturer into 0-3 μm and 5-10 μm particle size distributions. The measurements clearly show the effect of size distribution on the infrared backscatter coefficients as well as the dynamic nature of the size distribution for a population of aerosols. The test methodology and experimental results are presented.

  5. Study of MPLNET-Derived Aerosol Climatology over Kanpur, India, and Validation of CALIPSO Level 2 Version 3 Backscatter and Extinction Products

    NASA Technical Reports Server (NTRS)

    Misra, Amit; Tripathi, S. N.; Kaul, D. S.; Welton, Ellsworth J.

    2012-01-01

    The level 2 aerosol backscatter and extinction profiles from the NASA Micropulse Lidar Network (MPLNET) at Kanpur, India, have been studied from May 2009 to September 2010. Monthly averaged extinction profiles from MPLNET shows high extinction values near the surface during October March. Higher extinction values at altitudes of 24 km are observed from April to June, a period marked by frequent dust episodes. Version 3 level 2 Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) aerosol profile products have been compared with corresponding data from MPLNET over Kanpur for the above-mentioned period. Out of the available backscatter profiles, the16 profiles used in this study have time differences less than 3 h and distances less than 130 km. Among these profiles, four cases show good comparison above 400 m with R2 greater than 0.7. Comparison with AERONET data shows that the aerosol type is properly identified by the CALIOP algorithm. Cloud contamination is a possible source of error in the remaining cases of poor comparison. Another source of error is the improper backscatter-to-extinction ratio, which further affects the accuracy of extinction coefficient retrieval.

  6. Particle backscatter, extinction, and lidar ratio profiling with Raman lidar in south and north China

    SciTech Connect

    Tesche, Matthias; Ansmann, Albert; Mueller, Detlef; Althausen, Dietrich; Engelmann, Ronny; Hu Min; Zhang Yuanghang

    2007-09-01

    Aerosol Raman lidar observations of profiles of the particle extinction and backscatter coefficients and the respective extinction-to-backscatter ratio (lidar ratio) were performed under highly polluted conditions in the Pearl River Delta (PRD) in southern China in October 2004 and at Beijing during a clear period with moderately polluted to background aerosol conditions in January 2005. The anthropogenic haze in the PRD is characterized by volume light-extinction coefficients of particles ranging from approximately 200 to800 Mm-1 and lidar ratios mostly between 40 and 55 sr (average of47{+-}6 sr). Almost clean air masses were observed throughout the measurements of the Beijing campaign. These air masses originated from arid desert-steppe-like regions (greater Gobi area).Extinction values usually varied between 100 and300 Mm-1, and the lidar ratios were considerably lower (compared with PRD values) with values mostly from 30 to 45 sr (average of38{+-}7 sr). Gobi dust partly influenced the observations. Unexpectedly low lidar ratios of approximately 25 sr were found for a case of background aerosol with a low optical depth of 0.05. The low lidar ratios are consistent with Mie-scattering calculations applied to ground-based observations of particle size distributions.

  7. Aerosol speckle effects on atmospheric pulsed lidar backscattered signals

    NASA Technical Reports Server (NTRS)

    Murty, S. R.

    1989-01-01

    Lidar systems using atmospheric aerosols as targets exhibit return signal amplitude and power fluctuations which indicate speckle effects. The effects of refractive turbulence along the path on the aerosol speckle field propagation and on the decorrelation time are studied for coherent pulsed lidar systems.

  8. Intercomparison of Remote and Flight Level Measured Aerosol Backscatter Coefficient During GLOBE 2 Pacific Survey Mission

    NASA Technical Reports Server (NTRS)

    Cutten, D. R.; Spinhime, J. D.; Menzies, R. T.; Bowdle, D. A.; Srivastava, V.; Pueschel, R. F.; Clarke, A. D.; Rothermel, J.

    1998-01-01

    Aerosol backscatter coefficient data are examined from two local flights undertaken during NASA's GLObal Backscatter Experiment (GLOBE) in May - June, 1990. During each of these two flights the aircraft traversed different altitudes within a region of the atmosphere defined by the same set of latitude and longitude coordinates. This provides an ideal opportunity to allow flight level measured or modeled aerosol backscafter to be compared with pulsed lidar aerosol backscafter data that were obtained at these same altitudes either earlier or later than the flight level measurements. Aerosol backscafter comparisons were made at 1.06-, 9.11- and 9.25-mm wavelengths, using data from three lidar systems and two aerosol optical counters. The best agreement between all sensor's was found in the altitude region below 7 km where backscafter values were moderately high at all three wavelengths. Above this altitude the pulsed lidar backscafter data at 1.06- and 9.25-mm wavelengths were higher than the flight level data obtained from the CW lidar or derived from the optical counters. Possible reasons are offered to explain this discrepancy. During the Japan local flight, microphysics analysis revealed: (1) evidence of a strong advected seasalt aerosol plume from the marine boundary layer, and (2) where backscatter was low, the large lidar sampling volume included many large particles which were of different chemical composition to the small particle category sampled by the particle counters.

  9. Using Airborne High Spectral Resolution Lidar Data to Evaluate Combined Active Plus Passive Retrievals of Aerosol Extinction Profiles

    NASA Technical Reports Server (NTRS)

    Burton, S. P.; Ferrare, R. A.; Kittaka, C.; Hostetler, C. A.; Hair, J. W.; Obland, M. D.; Rogers, R. R.; Cook, A. L.; Haper, D. B.

    2008-01-01

    Aerosol extinction profiles are derived from backscatter data by constraining the retrieval with column aerosol optical thickness (AOT), for example from coincident MODIS observations and without reliance on a priori assumptions about aerosol type or optical properties. The backscatter data were acquired with the NASA Langley High Spectral Resolution Lidar (HSRL). The HSRL also simultaneously measures extinction independently, thereby providing an ideal data set for evaluating the constrained retrieval of extinction from backscatter. We will show constrained extinction retrievals using various sources of column AOT, and examine comparisons with the HSRL extinction measurements and with a similar retrieval using data from the CALIOP lidar on the CALIPSO satellite.

  10. Ozone and Aerosol Retrieval from Backscattered Ultraviolet Radiation

    NASA Technical Reports Server (NTRS)

    Bhartia, Pawan K.

    2012-01-01

    In this presentation we will discuss the techniques to estimate total column ozone and aerosol absorption optical depth from the measurements of back scattered ultraviolet (buv) radiation. The total ozone algorithm has been used to create a unique record of the ozone layer, spanning more than 3 decades, from a series of instruments (BUV, SBUV, TOMS, SBUV/2) flown on NASA, NOAA, Japanese and Russian satellites. We will discuss how this algorithm can be considered a generalization of the well-known Dobson/Brewer technique that has been used to process data from ground-based instruments for many decades, and how it differs from the DOAS techniques that have been used to estimate vertical column densities of a host of trace gases from data collected by GOME and SCIAMACHY instruments. The buv aerosol algorithm is most suitable for the detection of UV absorbing aerosols (smoke, desert dust, volcanic ash) and is the only technique that can detect aerosols embedded in clouds. This algorithm has been used to create a quarter century record of aerosol absorption optical depth using the buv data collected by a series of TOMS instruments. We will also discuss how the data from the OMI instrument launched on July 15, 2004 will be combined with data from MODIS and CALIPSO lidar data to enhance the accuracy and information content of satellite-derived aerosol measurements. The OMI and MODIS instruments are currently flying on EOS Aura and EOS Aqua satellites respectively, part of a constellation of satellites called the "A-train".

  11. Laser remote sensing of tropospheric aerosol over Southern Ireland using a backscatter Raman LIDAR

    NASA Astrophysics Data System (ADS)

    Ruth, Albert A.; Acheson, Karen; Apituley, Arnoud; Chaikovsky, Anatoli; Nicolae, Doina; Ortiz-Amezcua, Pablo; Stoyanov, Dimitar; Trickl, Thomas

    2016-04-01

    Raman backscatter coefficients, extinction coefficients and lidar ratios were measured with a ground based Raman lidar system at University College Cork, Ireland, during the periods of July 2012 - August 2012, April 2013 - December 2013 and March 2014 - May 2014. Statistical analysis of these parameters in this time provided information about seasonal effects of Raman backscatter coefficients and the altitude of the top of the planetary boundary layer. The mean of the altitude of the top of the planetary boundary layer over these time periods is 950 ± 302 m. The values are larger in summer, 1206 ± 367 m, than in winter, 735 m. The altitude of the top of the planetary boundary layer measured at Cork is lower than most EARLINET stations. Raman backscatter coefficients above and altitude of 2 km are highest in summer and spring where the values are greater than 0.28 Mm‑1 sr‑1. Winter values of Raman backscatter coefficient are less than 0.06 Mm‑1 sr‑1. These seasonal effects are consistent with most EARLINET stations. Large aerosol loads were detected in July 2013 due to a Canadian forest fire event. HYSPLIT air-mass back trajectory models were used to trace the origin of the detected aerosol layers. The aerosol forecast model, MACC, was used to further investigate and verify the propagation of the smoke. The Lidar ratio values and Klett and Raman backscatter coefficients at Cork, for the 4th July, the 7th to 9th of July and the 11th July were compared with observations at Cabauw, Minsk, Granada, Bucharest, Sofia and Garmisch. Lidar ratio values for the smoke detected at Cork were determined to be between 33 sr and 62 sr. The poster will discuss the seasonal changes of Raman backscatter coefficients and the altitude of the top of the planetary boundary layer at Cork. An investigation of a Canadian forest fire event measured at Cork will be compared with other data from the EARLINET database.

  12. Laser remote sensing of tropospheric aerosol over Southern Ireland using a backscatter Raman LIDAR

    NASA Astrophysics Data System (ADS)

    Ruth, Albert A.; Acheson, Karen; Apituley, Arnoud; Chaikovsky, Anatoli; Nicolae, Doina; Ortiz-Amezcua, Pablo; Stoyanov, Dimitar; Trickl, Thomas

    2016-04-01

    Raman backscatter coefficients, extinction coefficients and lidar ratios were measured with a ground based Raman lidar system at University College Cork, Ireland, during the periods of July 2012 - August 2012, April 2013 - December 2013 and March 2014 - May 2014. Statistical analysis of these parameters in this time provided information about seasonal effects of Raman backscatter coefficients and the altitude of the top of the planetary boundary layer. The mean of the altitude of the top of the planetary boundary layer over these time periods is 950 ± 302 m. The values are larger in summer, 1206 ± 367 m, than in winter, 735 m. The altitude of the top of the planetary boundary layer measured at Cork is lower than most EARLINET stations. Raman backscatter coefficients above and altitude of 2 km are highest in summer and spring where the values are greater than 0.28 Mm-1 sr-1. Winter values of Raman backscatter coefficient are less than 0.06 Mm-1 sr-1. These seasonal effects are consistent with most EARLINET stations. Large aerosol loads were detected in July 2013 due to a Canadian forest fire event. HYSPLIT air-mass back trajectory models were used to trace the origin of the detected aerosol layers. The aerosol forecast model, MACC, was used to further investigate and verify the propagation of the smoke. The Lidar ratio values and Klett and Raman backscatter coefficients at Cork, for the 4th July, the 7th to 9th of July and the 11th July were compared with observations at Cabauw, Minsk, Granada, Bucharest, Sofia and Garmisch. Lidar ratio values for the smoke detected at Cork were determined to be between 33 sr and 62 sr. The poster will discuss the seasonal changes of Raman backscatter coefficients and the altitude of the top of the planetary boundary layer at Cork. An investigation of a Canadian forest fire event measured at Cork will be compared with other data from the EARLINET database.

  13. Backscatter laser depolarization studies of simulated stratospheric aerosols - Crystallized sulfuric acid droplets

    NASA Technical Reports Server (NTRS)

    Sassen, Kenneth; Zhao, Hongjie; Yu, Bing-Kun

    1989-01-01

    The optical depolarizing properties of simulated stratospheric aerosols were studied in laboratory laser (0.633 micrometer) backscattering experiments for application to polarization lidar observations. Clouds composed of sulfuric acid solution droplets, some treated with ammonia gas, were observed during evaporation. The results indicate that the formation of minute ammonium sulfate particles from the evaporation of acid droplets produces linear depolarization ratios of beta equivalent to 0.02, but beta equivalent to 0.10 to 0.15 are generated from aged acid cloud aerosols and acid droplet crystalization effects following the introduction of ammonia gas into the chamber. It is concluded that partially crystallized sulfuric acid droplets are a likely candidate for explaining the lidar beta equivalent to 0.10 values that have been observed in the lower stratosphere in the absence of the relatively strong backscattering from homogeneous sulfuric acid droplet (beta equivalent to 0) or ice crystal (beta equivalent to 0.5) clouds.

  14. Backscatter laser depolarization studies of simulated stratospheric aerosols: crystallized sulfuric acid droplets.

    PubMed

    Sassen, K; Zhao, H; Yu, B K

    1989-08-01

    The optical depolarizing properties of simulated stratospheric aerosols were studied in laboratory laser (0.633 microm) backscattering experiments for application to polarization lidar observations. Clouds composed of sulfuric acid solution droplets, some treated with ammonia gas, were observed during evaporation. The results indicate that the formation of minute ammonium sulfate particles from the evaporation of acid droplets produces linear depolarization ratios of delta approximately 0.02, but delta approximately 0.10-0.15 are generated from acid droplet crystallization effects associated with recycled aerosols and the introduction of ammonia gas into the chamber. It is concluded that partially crystallized sulfuric acid droplets are a likely candidate for explaining the lidar delta approximately 0.10 values that have been observed in the lower stratosphere in the absence of the relatively strong backscattering from homogeneous sulfuric acid droplet (delta approximately 0) or ice crystal (delta approximately 0.5) clouds.

  15. Backscatter laser depolarization studies of simulated stratospheric aerosols: Crystallized sulfuric acid droplets

    NASA Technical Reports Server (NTRS)

    Sassen, Kenneth; Zhao, Hongjie; Yu, Bing-Kun

    1988-01-01

    The optical depolarizing properties of simulated stratospheric aerosols were studied in laboratory laser (0.633 micrometer) backscattering experiments for application to polarization lidar observations. Clouds composed of sulfuric acid solution droplets, some treated with ammonia gas, were observed during evaporation. The results indicate that the formation of minute ammonium sulfate particles from the evaporation of acid droplets produces linear depolarization ratios of beta equivalent to 0.02, but beta equivalent to 0.10 to 0.15 are generated from aged acid cloud aerosols and acid droplet crystallization effects following the introduction of ammonia gas into the chamber. It is concluded that partially crystallized sulfuric acid droplets are a likely candidate for explaining the lidar beta equivalent to 0.10 values that have been observed in the lower stratosphere in the absence of the relatively strong backscattering from homogeneous sulfuric acid droplet (beta equivalent to 0) or ice crystal (beta equivalent to 0.5) clouds.

  16. A tunable coherent CO2 lidar for measurements of atmospheric aerosol backscatter and attenuation

    NASA Technical Reports Server (NTRS)

    Menzies, R. T.

    1983-01-01

    A coherent laser radar system using a grating-tunable, injection-locked TEA-CO2 transmitter is being used to measure the altitude dependence of atmospheric aerosol backscatter and attenuation at a variety of CO2 laser wavelengths in the 9-11 micron region. Injection control of the TEA-CO2 laser allows one to obtain Single-Longitudinal-Mode (SLM) pulses which will follow the frequency of the injected radiation if the TEA laser cavity length is adjusted so that a cavity resonance is in proximity with the injected signal frequency, and if various additional conditions are satisfied. Requirements for generation of SLM pulses in this manner from a TEA CO2 laser with an unstable resonator cavity will be discussed. Procedures used for quantitative range-gated measurements of aerosol backscatter and attenuation will also be discussed.

  17. Variability of aerosol and spectral lidar and backscatter and extinction ratios of key aerosol types derived from selected Aerosol Robotic Network locations

    NASA Astrophysics Data System (ADS)

    Cattrall, Christopher; Reagan, John; Thome, Kurt; Dubovik, Oleg

    2005-05-01

    The lidar (extinction-to-backscatter) ratios at 0.55 and 1.02 μm and the spectral lidar, extinction, and backscatter ratios of climatically relevant aerosol species are computed on the basis of selected retrievals of aerosol properties from 26 Aerosol Robotic Network (AERONET) sites across the globe. The values, obtained indirectly from sky radiance and solar transmittance measurements, agree very well with values from direct observations. Low mean values of the lidar ratio, Sa, at 0.55 μm for maritime (27 sr) aerosols and desert dust (42 sr) are clearly distinguishable from biomass burning (60 sr) and urban/industrial pollution (71 sr). The effects of nonsphericity of mineral dust are shown, demonstrating that particle shape must be taken into account in any spaceborne lidar inversion scheme. A new aerosol model representing pollution over Southeast Asia is introduced since lidar (58 sr), color lidar, and extinction ratios in this region are distinct from those over other urban/industrial centers, owing to a greater number of large particles relative to fine particles. This discrimination promises improved estimates of regional climate forcing by aerosols containing black carbon and is expected to be of utility to climate modeling and remote sensing communities. The observed variability of the lidar parameters, combined with current validated aerosol data products from Moderate Resolution Imaging Spectroradiometer (MODIS), will afford improved accuracy in the inversion of spaceborne lidar data over both land and ocean.

  18. Evolution of the Pinatubo volcanic aerosol column above Pasadena, California observed with a mid-infrared backscatter lidar

    NASA Technical Reports Server (NTRS)

    Tratt, David M.; Menzies, Robert T.

    1995-01-01

    The evolution of the volcanic debris plume originating from the June 1991 eruption of Mt. Pinatubo has been monitored since its genesis using a ground-based backscatter lidar facility sited at the Jet Propulsion Laboratory (JPL). Both absolute and relative pre- and post-Pinatubo backscatter observations are in accord with Mie scattering projections based on measured aerosol particle size distributions reported in the literature. The post-Pinatubo column-integrated backscatter coefficient peaked approximately 400 days after the eruption, and the observed upper boundary of the aerosol column subsided at a rate of approximately 200 m/mon.

  19. Use of ceilometers for aerosol profile measurements: a comment from AD-Net

    NASA Astrophysics Data System (ADS)

    Jin, Yoshitaka; Kai, Kenji; Kawai, Kei; Sugimoto, Nobuo; Nishizawa, Tomoaki; Matsui, Ichiro; Shimizu, Atsushi; Batdorj, Dashdondog

    2014-11-01

    Ceilometer instruments are simple backscatter lidar systems and are usually set in airports for detecting the base of clouds. The instrument can also measure aerosol vertical distribution. Since ceilometers barely detect the molecular backscatter signals, retrieval of aerosol optical properties is an issue. This study investigates applicability of ceilometers to retrieval of optical properties. We make an idealized signal profile with the lidar ratio of 50 sr and calculate the retrieval errors caused by 30% errors of lidar ratio. In the forward inversion, useable (small error) optical properties are backscattering coefficients and the retrieval errors are less than 15% if the aerosol optical depth (AOD) is less than 0.2. The initial backscattering coefficients must be determined from other instruments (e.g., multi-wavelength lidar). Whereas in the backward inversion, if the AOD of idealized signals is larger than 1.5, extinction coefficients converge to the true value (within 5% errors), regardless of lidar ratios and initial conditions. Since there is no need for the system constant or molecular backscatter in this method, ceilometers can be an effective tool for retrieving extinction coefficients of dense aerosols in East Asia.

  20. Optical properties of different aerosol types: seven years of combined Raman- elastic backscatter lidar measurements in Thessaloniki, Greece

    NASA Astrophysics Data System (ADS)

    Giannakaki, E.; Balis, D. S.; Amiridis, V.; Zerefos, C.

    2009-11-01

    We present our combined Raman/elastic backscatter lidar observations which were carried out at the EARLINET station of Thessaloniki, Greece, during the period 2001-2007. The largest optical depths are observed for Saharan dust and smoke aerosol loads. For "local" and "continental polluted" aerosols the measurements indicate moderate aerosol loads. However, measurements associated with the "local" path show lower values of free tropospheric contribution (37% versus 46% for "continental polluted") and thus, enhanced aerosol load within the Planetary Boundary Layer. The lowest value of aerosol optical depth is observed for "continental clean" aerosols. The largest lidar ratios, of the order of 70 sr are found for biomass burning aerosols. A significant and distinct correlation between lidar ratio and backscatter related Ångström exponent values was estimated for well defined aerosol categories, which provides a statistical measure of the lidar ratio's dependency on aerosol-size, which is a useful tool for elastic lidar systems. Scatter plot between lidar ratio values and Ångström exponent values for "local" and "continental polluted" aerosols does not show a significant correlation, with a large variation in both parameters possibly due to variable absorption characteristics of these aerosols. Finally for "clean continental" aerosols we found constantly low lidar ratios almost independent of size.

  1. Airborne high spectral resolution lidar for measuring aerosol extinction and backscatter coefficients.

    PubMed

    Esselborn, Michael; Wirth, Martin; Fix, Andreas; Tesche, Matthias; Ehret, Gerhard

    2008-01-20

    An airborne high spectral resolution lidar (HSRL) based on an iodine absorption filter and a high-power frequency-doubled Nd:YAG laser has been developed to measure backscatter and extinction coefficients of aerosols and clouds. The instrument was operated aboard the Falcon 20 research aircraft of the German Aerospace Center (DLR) during the Saharan Mineral Dust Experiment in May-June 2006 to measure optical properties of Saharan dust. A detailed description of the lidar system, the analysis of its data products, and measurements of backscatter and extinction coefficients of Saharan dust are presented. The system errors are discussed and airborne HSRL results are compared to ground-based Raman lidar and sunphotometer measurements.

  2. Use of rotational Raman measurements in multiwavelength aerosol lidar for evaluation of particle backscattering and extinction

    NASA Astrophysics Data System (ADS)

    Veselovskii, I.; Whiteman, D. N.; Korenskiy, M.; Suvorina, A.; Pérez-Ramírez, D.

    2015-10-01

    Vibrational Raman scattering from nitrogen is commonly used in aerosol lidars for evaluation of particle backscattering (β) and extinction (α) coefficients. However, at mid-visible wavelengths, particularly in the daytime, previous measurements have possessed low signal-to-noise ratio. Also, vibrational scattering is characterized by a significant frequency shift of the Raman component, so for the calculation of α and β information about the extinction Ångström exponent is needed. Simulation results presented in this study demonstrate that ambiguity in the choice of Ångström exponent can be the a significant source of uncertainty in the calculation of backscattering coefficients when optically thick aerosol layers are considered. Both of these issues are addressed by the use of pure-rotational Raman (RR) scattering, which is characterized by a higher cross section compared to nitrogen vibrational scattering, and by a much smaller frequency shift, which essentially removes the sensitivity to changes in the Ångström exponent. We describe a practical implementation of rotational Raman measurements in an existing Mie-Raman lidar to obtain aerosol extinction and backscattering at 532 nm. A 2.3 nm width interference filter was used to select a spectral range characterized by low temperature sensitivity within the anti-Stokes branch of the RR spectrum. Simulations demonstrate that the temperature dependence of the scattering cross section does not exceed 1.5 % in the 230-300 K range, making correction for this dependence quite easy. With this upgrade, the NASA GSFC multiwavelength Raman lidar has demonstrated useful α532 measurements and was used for regular observations. Examples of lidar measurements and inversion of optical data to the particle microphysics are given.

  3. Use of Lidar Derived Optical Extinction and Backscattering Coefficients Near Cloud Base to Explore Aerosol-Cloud Interactions

    NASA Astrophysics Data System (ADS)

    Han, Zaw; Wu, Yonhgua; Gross, Barry; Moshary, Fred

    2016-06-01

    Combination of microwave radiometer (MWR) and mutlifilter rotating shadowband radiometer (MFRSR) measurement data together with SBDART radiative transfer model to compute cloud optical depth (COD) and cloud droplet effective radius (Reff). Quantify the first aerosol indirect effect using calculated Reff and aerosol extinction from Raman lidar measurement in urban coastal region. Illustrate comparison between ground-based and satellite retrievals. Demonstrate relationship between surface aerosol (PM2.5) loading and Reff. We also explain the sensitivity of aerosol-cloud-index (ACI) depend on the aerosol layer from cloud base height. Potential used of less noisy elastic backscattering to calculate the ACI instead of using Raman extinction. We also present comparison of elastic backscattering and Raman extinction correlation to Reff.

  4. Backscattering measurements of atmospheric aerosols at CO2 laser wavelengths: implications of aerosol spectral structure on differential-absorption lidar retrievals of molecular species.

    PubMed

    Ben-David, A

    1999-04-20

    The volume backscattering coefficients of atmospheric aerosol were measured with a tunable CO2 lidar system at various wavelengths in Utah (a desert environment) along a horizontal path a few meters above the ground. In deducing the aerosol backscattering, a deconvolution (to remove the smearing effect of the long CO2 lidar pulse and the lidar limited bandwidth) and a constrained-slope method were employed. The spectral shape beta(lambda) was similar for all the 13 measurements during a 3-day period. A mean aerosol backscattering-wavelength dependence beta(lambda) was computed from the measurements and used to estimate the error Delta(CL) (concentration-path-length product) in differential-absorption lidar measurements for various gases caused by the systematic aerosol differential backscattering and the error that is due to fluctuations in the aerosol backscattering. The water-vapor concentration-path-length product CL and the average concentration C = /L for a path length L computed from the range-resolved lidar measurements is consistently in good agreement with the water-vapor concentration measured by a meteorological station. However, I was unable to deduce, reliably, the range-resolved water-vapor concentration C(r), which is the derivative of the range-dependent product CL, because of the effect of residual noise caused mainly by errors in the deconvolved lidar measurements.

  5. Aerosol backscatter measurements at 10. 6 micrometers with airborne and ground-based CO sub 2 Doppler lidars over the Colorado high plains. 1. Lidar intercomparison

    SciTech Connect

    Bowdle, D.A. ); Rothermel, J. ); Vaughan, J.M.; Brown, D.W. ); Post, M.J. )

    1991-03-20

    An airborne continuous wave (CW) focused CO{sub 2} Doppler lidar and a ground-based pulsed CO{sub 2} Doppler lidar were used to obtain seven pairs of comparative measurements of tropospheric aerosol backscatter profiles at 10.6 {mu}m wavelength, near Denver, Colorado, during a 20-day period in July 1982. In regions of uniform backscatter the two lidars show good agreement, with differences usually less than {approximately}50% near 8-km altitude and less than a factor of 2 or 3 elsewhere but with the pulsed lidar often lower than the CW lidar. Near sharp backscatter gradients the two lidars show poorer agreement, with the pulsed lidar usually higher than the CW lidar. Most discrepancies arise from a combination of atmospheric factors and instrument factors, particularly small-scale areal and temporal backscatter heterogeneity above the planetary boundary layer, unusual large-scale vertical backscatter structure in the upper troposphere and lower stratosphere, and differences in the spatial resolution, detection threshold, and noise estimation for the two lidars.

  6. Using Airborne High Spectral Resolution Lidar Data to Evaluate Combined Active Plus Passive Retrievals of Aerosol Extinction Profiles

    NASA Technical Reports Server (NTRS)

    Burton, S. P.; Ferrare, R. A.; Hostetler, C. A.; Hair, J. W.; Kittaka, C.; Vaughn, M. A.; Remer, L. A.

    2010-01-01

    We derive aerosol extinction profiles from airborne and space-based lidar backscatter signals by constraining the retrieval with column aerosol optical thickness (AOT), with no need to rely on assumptions about aerosol type or lidar ratio. The backscatter data were acquired by the NASA Langley Research Center airborne High Spectral Resolution Lidar (HSRL) and by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument on the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite. The HSRL also simultaneously measures aerosol extinction coefficients independently using the high spectral resolution lidar technique, thereby providing an ideal data set for evaluating the retrieval. We retrieve aerosol extinction profiles from both HSRL and CALIOP attenuated backscatter data constrained with HSRL, Moderate-Resolution Imaging Spectroradiometer (MODIS), and Multiangle Imaging Spectroradiometer column AOT. The resulting profiles are compared with the aerosol extinction measured by HSRL. Retrievals are limited to cases where the column aerosol thickness is greater than 0.2 over land and 0.15 over water. In the case of large AOT, the results using the Aqua MODIS constraint over water are poorer than Aqua MODIS over land or Terra MODIS. The poorer results relate to an apparent bias in Aqua MODIS AOT over water observed in August 2007. This apparent bias is still under investigation. Finally, aerosol extinction coefficients are derived from CALIPSO backscatter data using AOT from Aqua MODIS for 28 profiles over land and 9 over water. They agree with coincident measurements by the airborne HSRL to within +/-0.016/km +/- 20% for at least two-thirds of land points and within +/-0.028/km +/- 20% for at least two-thirds of ocean points.

  7. Two-wavelength backscattering lidar for stand off detection of aerosols

    NASA Astrophysics Data System (ADS)

    Mierczyk, Zygmunt; Zygmunt, Marek; Gawlikowski, Andrzej; Gietka, Andrzej; Kaszczuk, Miroslawa; Knysak, Piotr; Mlodzianko, Andrzej; Muzal, Michal; Piotrowski, Wiesław; Wojtanowski, Jacek

    2008-10-01

    Following article presents LIDAR for stand off detection of aerosols which was constructed in Institute of Optoelectronics in Military University of Technology. LIDAR is a DISC type system (DIfferential SCattering) and is based on analysis of backscattering signal for two wavelengths (λ1 = 1064 nm and λ2 = 532 nm) - the first and the second harmonic of Nd:YAG laser. Optical receiving system is consisted of aspherical mirror lens, two additional mirrors and a system of interference filters. In detection system of LIDAR a silicon avalanche photodiode and two different amplifiers were used. Whole system is mounted on a specialized platform designed for possibility of LIDAR scanning movements. LIDAR is computer controlled. The compiled software enables regulation of the scanning platform work, gain control, and control of data processing and acquisition system. In the article main functional elements of LIDAR are shown and typical parameters of system work and construction are presented. One presented also first results of research with use of LIDAR. The aim of research was to detect and characterize scattering aerosol, both natural and anthropogenic one. For analyses of natural aerosols, cumulus cloud was used. For analyses of anthropogenic aerosols one used three various pyrotechnic mixtures (DM11, M2, M16) which generate smoke of different parameters. All scattering centers were firstly well described and theoretical analyses were conducted. Results of LIDAR research were compared with theoretical analyses and general conclusions concerning correctness of LIDAR work and its application were drawn.

  8. Extinction-to-Backscatter Ratios of Lofted Aerosol Layers Observed During the First Three Months of CALIPSO Measurements

    NASA Technical Reports Server (NTRS)

    Omar, Ali H.; Vaughan, Mark A.; Liu, Zhaoyan; Hu, Yongxiang; Reagan, John A.; Winker, David M.

    2007-01-01

    Case studies from the first three months of the Cloud and Aerosol Lidar and Infrared Pathfinder Spaceborne Observations (CALIPSO) measurements of lofted aerosol layers are analyzed using transmittance [Young, 1995] and two-wavelength algorithms [Vaughan et al., 2004] to determine the aerosol extinction-to-backscatter ratios at 532 and 1064 nm. The transmittance method requires clear air below the layer so that the transmittance through the layer can be determined. Suitable scenes are selected from the browse images and clear air below features is identified by low 532 nm backscatter signal and confirmed by low depolarization and color ratios. The transmittance and two-wavelength techniques are applied to a number of lofted layers and the extinction-to-backscatter ratios are compared with values obtained from the CALIPSO aerosol models [Omar et al., 2004]. The results obtained from these studies are used to adjust the aerosol models and develop observations based extinction-to-backscatter ratio look-up tables and phase functions. Values obtained by these techniques are compared to Sa determinations using other independent methods with a goal of developing probability distribution functions of aerosol type-specific extinction to backscatter ratios. In particular, the results are compared to values determined directly by the High Spectral Resolution Lidar (HSRL) during the CALIPSO CloudSat Validation Experiments (CCVEX) and Sa determined by the application of the two-wavelength lidar Constrained Ratio Aerosol Model-fit (CRAM) retrieval approach [Cattrall et al., 2005; Reagan et al., 2004] to the HSRL data. The results are also compared to values derived using the empirical relationship between the multiple-scattering fraction and the linear depolarization ratio by using Monte Carlo simulations of water clouds [Hu et al., 2006].

  9. Scanning Backscatter Lidar Observations for Characterizing 4-D Cloud and Aerosol Fields to Improve Radiative Transfer Parameterizations

    NASA Technical Reports Server (NTRS)

    Schwemmer, Geary K.; Miller, David O.

    2005-01-01

    dimensions. HARLIE was used in a ground-based configuration in several recent field campaigns. Principal data products include aerosol backscatter profiles, boundary layer heights, entrainment zone thickness, cloud fraction as a function of altitude and horizontal wind vector profiles based on correlating the motions of clouds and aerosol structures across portions of the scan. Comparisons will be made between various cloud detecting instruments to develop a baseline performance metric.

  10. Near Real Time Vertical Profiles of Clouds and Aerosols from the Cloud-Aerosol Transport System (CATS) on the International Space Station

    NASA Astrophysics Data System (ADS)

    Yorks, J. E.; McGill, M. J.; Nowottnick, E. P.

    2015-12-01

    Plumes from hazardous events, such as ash from volcanic eruptions and smoke from wildfires, can have a profound impact on the climate system, human health and the economy. Global aerosol transport models are very useful for tracking hazardous plumes and predicting the transport of these plumes. However aerosol vertical distributions and optical properties are a major weakness of global aerosol transport models, yet a key component of tracking and forecasting smoke and ash. The Cloud-Aerosol Transport System (CATS) is an elastic backscatter lidar designed to provide vertical profiles of clouds and aerosols while also demonstrating new in-space technologies for future Earth Science missions. CATS has been operating on the Japanese Experiment Module - Exposed Facility (JEM-EF) of the International Space Station (ISS) since early February 2015. The ISS orbit provides more comprehensive coverage of the tropics and mid-latitudes than sun-synchronous orbiting sensors, with nearly a three-day repeat cycle. The ISS orbit also provides CATS with excellent coverage over the primary aerosol transport tracks, mid-latitude storm tracks, and tropical convection. Data from CATS is used to derive properties of clouds and aerosols including: layer height, layer thickness, backscatter, optical depth, extinction, and depolarization-based discrimination of particle type. The measurements of atmospheric clouds and aerosols provided by the CATS payload have demonstrated several science benefits. CATS provides near-real-time observations of cloud and aerosol vertical distributions that can be used as inputs to global models. The infrastructure of the ISS allows CATS data to be captured, transmitted, and received at the CATS ground station within several minutes of data collection. The CATS backscatter and vertical feature mask are part of a customized near real time (NRT) product that the CATS processing team produces within 6 hours of collection. The continuous near real time CATS data

  11. Relationships between optical extinction, backscatter and aerosol surface and volume in the stratosphere following the eruption of Mt. Pinatubo

    SciTech Connect

    Brock, C.A.; Jonsson, H.H.; Wilson, J.C. ); Dye, J.E.; Baumgardner, D.; Borrmann, S.; Pitts, M.C.; Osborn, M.T.; DeCoursey, R.J.; Woods, D.C.

    1993-11-19

    The eruption of the Mt. Pinatubo volcano in the Philippines in June 1991 has resulted in increases in the surface and mass concentrations of aerosol particles in the lower stratosphere. Airborne measurements made at midlatitudes between 15 and 21 km from August 1991 to March 1992 show that, prior to December 1991, the Pinatubo aerosol cloud varied widely in microphysical properties such as size distribution, number, surface and volume concentration and was also spatially variable. Aerosol surface area concentration was found to be highly correlated to extinction at visible and near-infrared wavelengths throughout the measurement period. Similarly, backscatter at common lidar wavelengths was a good predictor of aerosol volume concentrations. These results support the use of satellite extinction measurements to estimate aerosol surface and of lidar measurements to estimate aerosol volume or mass if temporal changes in the relationships between the variables are considered. 23 refs., 3 figs., 1 tab.

  12. Analysis of the performance of a coherent pulsed fiber lidar for aerosol backscatter applications.

    PubMed

    Pearson, Guy N; Roberts, P John; Eacock, Justin R; Harris, Michael

    2002-10-20

    The antenna and the Doppler estimation characteristics of a coherent pulsed lidar intended for short-range aerosol backscatter applications have been analyzed. The system used fiber-optic interconnects and operated at a wavelength of 1.548 microm. The range dependence of the signal for various bistatic and monostatic antenna configurations has been determined. The system operated in a low-pulse-energy, high-pulse-repetition-rate mode, and the Doppler estimates from the return signal were achieved with a multipulse accumulation procedure. The expected performance of the accumulation in this low-photocount regime was compared with the data obtained from the system, and a reasonable level of agreement was demonstrated. PMID:12396197

  13. Aerosol measurements over the Pacific Ocean in support of the IR aerosol backscatter program

    NASA Technical Reports Server (NTRS)

    Prospero, Joseph M.; Savoie, Dennis L.

    1995-01-01

    The major efforts under NASA contract NAG8-841 included: (1) final analyses of the samples collected during the first GLOBE survey flight that occurred in November 1989 and collections and analysis of aerosol samples during the second GLOBE survey flight in May and June 1990. During the first GLOBE survey flight, daily samples were collected at four stations (Midway, Rarotonga, American Samoa, and Norfolk Island) throughout the month of November 1989. Weekly samples were collected at Shemya, Alaska, and at Karamea, New Zealand. During the second GLOBE survey flight, daily samples were collected at Midway, Oahu, American Samoa, Rarotonga, and Norfolk Island; weekly samples were collected at Shemya. These samples were all analyzed for sodium (sea-salt), chloride, nitrate, sulfate, and methanesulfonate at the University of Miami and for aluminum at the University of Rhode Island (under a subcontract). (2) Samples continued to be collected on a weekly basis at all stations during the periods between and after the survey flights. These weekly samples were also analyzed at the University of Miami for the suite of water-soluble species. (3) In August 1990, the results obtained from the above studies were submitted to the appropriate personnel at NASA Marshall Space Flight Center to become part of the GLOBE data base for comparison with data from instruments used aboard the aircraft. In addition, the data will be compared with data previously obtained at these stations as part of the Sea-Air Exchange (SEAREX) Program. This comparison will provide valuable information on the representativeness of the periods in terms of the longer term aerosol climatology over the Pacific Ocean. (4) Several publications have been written using data from this grant. The data will continue to be used in the future as part of a continuing investigation of the long-term trends and interannual variations in aerosol species concentrations over the Pacific Ocean.

  14. Intercomparison of Pulsed Lidar Data with Flight Level CW Lidar Data and Modeled Backscatter from Measured Aerosol Microphysics Near Japan and Hawaii

    NASA Technical Reports Server (NTRS)

    Cutten, D. R.; Spinhirne, J. D.; Menzies, R. T.; Bowdle, D. A.; Srivastava, V.; Pueschel, R. F.; Clarke, A. D.; Rothermel, J.

    1998-01-01

    Aerosol backscatter coefficient data were examined from two nights near Japan and Hawaii undertaken during NASA's Global Backscatter Experiment (GLOBE) in May-June 1990. During each of these two nights the aircraft traversed different altitudes within a region of the atmosphere defined by the same set of latitude and longitude coordinates. This provided an ideal opportunity to allow flight level focused continuous wave (CW) lidar backscatter measured at 9.11-micron wavelength and modeled aerosol backscatter from two aerosol optical counters to be compared with pulsed lidar aerosol backscatter data at 1.06- and 9.25-micron wavelengths. The best agreement between all sensors was found in the altitude region below 7 km, where backscatter values were moderately high at all three wavelengths. Above this altitude the pulsed lidar backscatter data at 1.06- and 9.25-micron wavelengths were higher than the flight level data obtained from the CW lidar or derived from the optical counters, suggesting sample volume effects were responsible for this. Aerosol microphysics analysis of data near Japan revealed a strong sea-salt aerosol plume extending upward from the marine boundary layer. On the basis of sample volume differences, it was found that large particles were of different composition compared with the small particles for low backscatter conditions.

  15. Raman lidar profiling of water vapor and aerosols over the ARM SGP Site

    SciTech Connect

    Ferrare, R.A.

    2000-01-09

    The authors have developed and implemented automated algorithms to retrieve profiles of water vapor mixing ratio, aerosol backscattering, and aerosol extinction from Southern Great Plains (SGP) Cloud and Radiation Testbed (CART) Raman Lidar data acquired during both daytime and nighttime operations. The Raman lidar sytem is unique in that it is turnkey, automated system designed for unattended, around-the-clock profiling of water vapor and aerosols. These Raman lidar profiles are important for determining the clear-sky radiative flux, as well as for validating the retrieval algorithms associated with satellite sensors. Accurate, high spatial and temporal resolution profiles of water vapor are also required for assimilation into mesoscale models to improve weather forecasts. The authors have also developed and implemented routines to simultaneously retrieve profiles of relative humidity. These routines utilize the water vapor mixing ratio profiles derived from the Raman lidar measurements together with temperature profiles derived from a physical retrieval algorithm that uses data from a collocated Atmospheric Emitted Radiance Interferometer (AERI) and the Geostationary Operational Environmental Satellite (GOES). These aerosol and water vapor profiles (Raman lidar) and temperature profiles (AERI+GOES) have been combined into a single product that takes advantage of both active and passive remote sensors to characterize the clear sky atmospheric state above the CART site.

  16. Application of HARLIE Measurements in Mesoscale Studies: Measurements of Aerosol Backscatter and Winds During A Gust Front

    NASA Technical Reports Server (NTRS)

    Demoz, Belay; Miller, David; Schwemmer, Geary; Starr, David OC (Technical Monitor)

    2001-01-01

    Lidar atmospheric systems have required large telescope for receiving atmospheric backscatter signals. Thus, the relative complexity in size and ease of operation has limited their wider use in the atmospheric science and meteorology community. The Holographic Airborne Rotating Lidar Instrument Experiment (HARLIE) uses a scanning holographic receiver and demonstrates that these issues can be overcome. HARLIE participated at the DOE-ARM Southern Great Plains site (CART) during the Water Vapor Intensive Operation Period (WVIOP2000) held September-October 2000. It provided exceptional high temporal and spatial resolution measurements of aerosol and cloud backscatter in three dimensions. HARLIE recorded over 110 hours of data were recorded on 16 days between 17 September and 6 October 2000. Placed in a ground-based trailer for upward looking scanning measurements of clouds and aerosols, HARLIE provided a unique record of time-resolved atmospheric backscatter at 1-micron wavelength. The conical scanning lidar measures atmospheric backscatter on the surface of an inverted 90 degree (full angle) cone up to an altitude of 20 km, 360-degree scans having spatial resolutions of 20 meters in the vertical and 1 degree in azimuth were obtained every 36 seconds during the daily, operating period. In this study we present highlights of HARLIE-based measurements of the boundary layer and cloud parameters as well as atmospheric wind vectors where there is sufficiently resolved structure in the backscatter. In particular we present data and discussions from a bore-front case observed on 23 September 2000.

  17. Comparison of aerosol backscatter and wind field estimates from the REAL and the SAMPLE

    NASA Astrophysics Data System (ADS)

    Mayor, Shane D.; Dérian, Pierre; Mauzey, Christopher F.; Spuler, Scott M.; Ponsardin, Patrick; Pruitt, Jeff; Ramsey, Darrell; Higdon, Noah S.

    2015-09-01

    Although operating at the same near-infrared 1.5- m wavelength, the Raman-shifted Eye-safe Aerosol Lidar (REAL) and the Scanning Aerosol Micro-Pulse Lidar-Eye-safe (SAMPLE) are very different in how they generate and detect laser radiation. We present results from an experiment where the REAL and the SAMPLE were operated side-by-side in Chico, California, in March of 2015. During the non-continuous, eleven day test period, the SAMPLE instrument was operated at maximum pulse repetition frequency (15 kHz) and integrated over the interpulse period of the REAL (0.1 s). Operation at the high pulse repetition frequency resulted in second trip echoes which contaminated portions of the data. The performance of the SAMPLE instrument varied with background brightness--as expected with a photon counting receiver|--yet showed equal or larger backscatter intensity signal to noise ratio throughout the intercomparison experiment. We show that a modest low-pass filter or smooth applied to the REAL raw waveforms (that have 5x higher range resolution) results in significant increases in raw signal-to-noise ratio and image signal-to-noise ratio--a measure of coherent aerosol feature content in the images resulting from the scans. Examples of wind fields and time series of wind estimates from both systems are presented. We conclude by reviewing the advantages and disadvantages of each system and sketch a plan for future research and development activities to optimize the design of future systems.

  18. Measurements of Aerosol Vertical Profiles and Optical Properties during INDOEX 1999 Using Micro-Pulse Lidars

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth J.; Voss, Kenneth J.; Quinn, Patricia K.; Flatau, Piotr J.; Markowicz, Krzysztof; Campbell, James R.; Spinhirne, James D.; Gordon, Howard R.; Johnson, James E.; Starr, David OC. (Technical Monitor)

    2001-01-01

    Micro-pulse lidar systems (MPL) were used to measure aerosol properties during the Indian Ocean Experiment (INDOEX) 1999 field phase. Measurements were made from two platforms: the NOAA ship RN Ronald H. Brown, and the Kaashidhoo Climate Observatory (KCO) in the Maldives. Sunphotometers were used to provide aerosol optical depths (AOD) needed to calibrate the MPL. This study focuses on the height distribution and optical properties (at 523 nm) of aerosols observed during the campaign. The height of the highest aerosols (top height) was calculated and found to be below 4 km for most of the cruise. The marine boundary layer (MBL) top was calculated and found to be less than 1 km. MPL results were combined with air mass trajectories, radiosonde profiles of temperature and humidity, and aerosol concentration and optical measurements. Humidity varied from approximately 80% near the surface to 50% near the top height during the entire cruise. The average value and standard deviation of aerosol optical parameters were determined for characteristic air mass regimes. Marine aerosols in the absence of any continental influence were found to have an AOD of 0.05 +/- 0.03, an extinction-to-backscatter ratio (S-ratio) of 33 +/- 6 sr, and peak extinction values around 0.05/km (near the MBL top). The marine results are shown to be in agreement with previously measured and expected values. Polluted marine areas over the Indian Ocean, influenced by continental aerosols, had AOD values in excess of 0.2, S-ratios well above 40 sr, and peak extinction values approximately 0.20/km (near the MBL top). The polluted marine results are shown to be similar to previously published values for continental aerosols. Comparisons between MPL derived extinction near the ship (75 m) and extinction calculated at ship-level using scattering measured by a nephelometer and absorption using a PSAP were conducted. The comparisons indicated that the MPL algorithm (using a constant S-ratio throughout the

  19. Atmospheric Backscatter Profiles at 765nm and 1572nm from Pulsed Lidar Measurements of CO2 and O2 Column Absorption from the 2013 ASCENDS Flight Campaign

    NASA Astrophysics Data System (ADS)

    Allan, G. R.; Riris, H.; Hasselbrack, W.; Rodriguez, M.; Ramanathan, A.; Sun, X.; Mao, J.; Abshire, J. B.

    2013-12-01

    We present height-resolved, range corrected, backscatter profiles from NASA GSFC's two-channel (CO2 & O2) sounder, an Integrated Path Differential Absorption (IPDA) lidar, which measures simultaneously both carbon dioxide & oxygen column absorptions. These backscatter profiles show clear evidence of multiple backscattering layers, clouds & aerosols, which allows for the identification of the Planetary Boundary Layer (PBL). The backscatter measurements enable sampling of the vertical distribution of CO2 in the atmosphere when broken & thin clouds are present & may help identify sources & sinks within the PBL as opposed to natural variations in the vertical distribution of CO2. The CO2 Sounder is an airborne pulsed lidar for active remote measurements of CO2 abundance & is a candidate for NASA's ASCENDS mission (Active Sensing of CO2 Emissions over Nights, Days & Seasons). The O2 channel measures atmospheric pressure in the same air column to calculate the dry mixing ratio of CO2. The lidars use a scanning, pulsed laser & fiber amplifier in a Master Oscillator Power Amplifier configuration to measure lineshape, range to scattering surface & backscatter profiles. The CO2 channel operates at 1572.335 nm. The O2 channel uses similar technology but frequency doubles the output from ~1530nm to the O2 A-band absorption around 765nm. Both lasers are scanned across the absorption feature of interest sampling the line at a fixed number of discrete wavelengths per scan around ~300 scans per second. The time-resolved return signal is detected by photon-counting detectors with a temporal resolution of a few nanoseconds. The CO2 channel uses a PMT while the O2 channel uses Single Photon Counting Modules. The detectors are fiber coupled to a 2m f10 Schmidt-Cassegrain telescope. The column density of the gas of interest is estimated from the differential optical depths of the scanned absorption using the IPDA technique & the optical path from the time of flight. A backscatter

  20. An Aerosol Extinction-to-Backscatter Ratio Database Derived from the NASA Micro-Pulse Lidar Network: Applications for Space-based Lidar Observations

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth J.; Campbell, James R.; Spinhime, James D.; Berkoff, Timothy A.; Holben, Brent; Tsay, Si-Chee; Bucholtz, Anthony

    2004-01-01

    Backscatter lidar signals are a function of both backscatter and extinction. Hence, these lidar observations alone cannot separate the two quantities. The aerosol extinction-to-backscatter ratio, S, is the key parameter required to accurately retrieve extinction and optical depth from backscatter lidar observations of aerosol layers. S is commonly defined as 4*pi divided by the product of the single scatter albedo and the phase function at 180-degree scattering angle. Values of S for different aerosol types are not well known, and are even more difficult to determine when aerosols become mixed. Here we present a new lidar-sunphotometer S database derived from Observations of the NASA Micro-Pulse Lidar Network (MPLNET). MPLNET is a growing worldwide network of eye-safe backscatter lidars co-located with sunphotometers in the NASA Aerosol Robotic Network (AERONET). Values of S for different aerosol species and geographic regions will be presented. A framework for constructing an S look-up table will be shown. Look-up tables of S are needed to calculate aerosol extinction and optical depth from space-based lidar observations in the absence of co-located AOD data. Applications for using the new S look-up table to reprocess aerosol products from NASA's Geoscience Laser Altimeter System (GLAS) will be discussed.

  1. The Cloud-Aerosol Transport System (CATS): a New Lidar for Aerosol and Cloud Profiling from the International Space Station

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth J.; McGill, Matthew J.; Yorks, John E.; Hlavka, Dennis L.; Hart, William D.; Palm, Stephen P.; Colarco, Peter R.

    2011-01-01

    Spaceborne lidar profiling of aerosol and cloud layers has been successfully implemented during a number of prior missions, including LITE, ICESat, and CALIPSO. Each successive mission has added increased capability and further expanded the role of these unique measurements in wide variety of applications ranging from climate, to air quality, to special event monitoring (ie, volcanic plumes). Many researchers have come to rely on the availability of profile data from CALIPSO, especially data coincident with measurements from other A-Train sensors. The CALIOP lidar on CALIPSO continues to operate well as it enters its fifth year of operations. However, active instruments have more limited lifetimes than their passive counterparts, and we are faced with a potential gap in lidar profiling from space if the CALIOP lidar fails before a new mission is operational. The ATLID lidar on EarthCARE is not expected to launch until 2015 or later, and the lidar component of NASA's proposed Aerosols, Clouds, and Ecosystems (ACE) mission would not be until after 2020. Here we present a new aerosol and cloud lidar that was recently selected to provide profiling data from the International Space Station (ISS) starting in 2013. The Cloud-Aerosol Transport System (CATS) is a three wavelength (1064, 532, 355 nm) elastic backscatter lidar with HSRL capability at 532 nm. Depolarization measurements will be made at all wavelengths. The primary objective of CATS is to continue the CALIPSO aerosol and cloud profile data record, ideally with overlap between both missions and EarthCARE. In addition, the near real time data capability of the ISS will enable CATS to support operational applications such as air quality and special event monitoring. The HSRL channel will provide a demonstration of technology and a data testbed for direct extinction retrievals in support of ACE mission development. An overview of the instrument and mission will be provided, along with a summary of the science

  2. Aerosol profiling using the ceilometer network of the German Meteorological Service

    NASA Astrophysics Data System (ADS)

    Flentje, H.; Heese, B.; Reichardt, J.; Thomas, W.

    2010-08-01

    The German Meteorological Service (DWD) operates about 52 lidar ceilometers within its synoptic observations network, covering Germany. These affordable low-power lidar systems provide spatially and temporally high resolved aerosol backscatter profiles which can operationally provide quasi 3-D distributions of particle backscatter intensity. Intentionally designed for cloud height detection, recent significant improvements allow following the development of the boundary layer and to detect denser particle plumes in the free tropospere like volcanic ash, Saharan dust or fire smoke. Thus the network builds a powerful aerosol plume alerting and tracking system. If auxiliary aerosol information is available, the particle backscatter coefficient, the extinction coefficient and even particle mass concentrations may be estimated, with however large uncertainties. Therefore, large synergistic benefit is achieved if the ceilometers are linked to existing lidar networks like EARLINET or integrated into WMO's envisioined Global Aerosol Lidar Observation Network GALION. To this end, we demonstrate the potential and limitations of ceilometer networks by means of three representative aerosol episodes over Europe, namely Sahara dust, Mediterranean fire smoke and, more detailed, the Icelandic Eyjafjoll volcano eruption from mid April 2010 onwards. The DWD (Jenoptik CHM15k) lidar ceilometer network tracked the Eyjafjoll ash layers over Germany and roughly estimated peak extinction coefficients and mass concentrations on 17 April of 4-6(± 2) 10-4 m-1 and 500-750(± 300) μg/m-3, respectively, based on co-located aerosol optical depth, nephelometer (scattering coefficient) and particle mass concentration measurements. Though large, the uncertainties are small enough to let the network suit for example as aviation advisory tool, indicating whether the legal flight ban threshold of presently 2 mg/m3 is imminent to be exceeded.

  3. Effect of particle settling on lidar profiles of long-range transported Saharan aerosols

    NASA Astrophysics Data System (ADS)

    Gasteiger, Josef; Groß, Silke

    2016-04-01

    A large amount of desert aerosol is transported in the Saharan Air Layer (SAL) westwards from Africa over the Atlantic Ocean. Lidar profiles of transported Saharan aerosol may contain some information about the vertically-resolved aerosol microphysics that could be used to characterize processes that affected the measured aerosol during transport. We present modelled lidar profiles of long-range transported Saharan aerosol assuming that initially the SAL is well-mixed and that there is no vertical mixing of air within the SAL as soon as it reaches the Atlantic. We consider Stokes gravitational settling of aerosol particles over the ocean. The lidar profiles are calculated using optical models for irregularly-shaped mineral dust particles assuming settling-induced particle removal as function of distance from the SAL top. Within the SAL we find a decrease of both the backscatter coefficients and the linear depolarization ratios with decreasing distance from the SAL top. For example, the linear depolarization ratio at a wavelength of 532nm decreases from 0.289 at 1000m to 0.256 at 200m and 0.215 at 100m below SAL top. We compare the modelled backscatter coefficients and linear depolarization ratios to ground-based lidar measurements performed during the SALTRACE field campaign in Barbados (Caribbean) and find agreement within the estimated uncertainties. We discuss the uncertainties of our modeling approach in our presentation. Assumed mineral dust particle shapes, assumed particle mixture properties, and assumptions about processes in the SAL over the continent and the ocean are important aspects to be considered. Uncertainties are relevant for the potential of lidar measurements of transported Saharan dust to learn something about processes occuring in the SAL during long-range transport. We also compare our modeling results to modeling results previously published in the literature.

  4. Doppler Lidar Measurements of Tropospheric Wind Profiles Using the Aerosol Double Edge Technique

    NASA Technical Reports Server (NTRS)

    Gentry, Bruce M.; Li, Steven X.; Mathur, Savyasachee; Korb, C. Laurence; Chen, Huailin

    2000-01-01

    The development of a ground based direct detection Doppler lidar based on the recently described aerosol double edge technique is reported. A pulsed, injection seeded Nd:YAG laser operating at 1064 nm is used to make range resolved measurements of atmospheric winds in the free troposphere. The wind measurements are determined by measuring the Doppler shift of the laser signal backscattered from atmospheric aerosols. The lidar instrument and double edge method are described and initial tropospheric wind profile measurements are presented. Wind profiles are reported for both day and night operation. The measurements extend to altitudes as high as 14 km and are compared to rawinsonde wind profile data from Dulles airport in Virginia. Vertical resolution of the lidar measurements is 330 m and the rms precision of the measurements is a low as 0.6 m/s.

  5. Retrieving seawater-backscattering profiles from coupling Raman and elastic lidar data.

    PubMed

    Malinka, Aleksey V; Zege, Eleonora P

    2004-07-01

    We propose a technique for retrieving seawater-backscattering profiles that is based on the joint use of elastic and Raman lidar returns. We suggest using two lidar channels: the Raman channel and the elastic channel with a light frequency equal to a half-sum of initial and Raman-shifted frequencies of the Raman channel. These specific wavelengths provide the same attenuation laws for elastic and Raman signals if absorption and scattering spectra can be approximated by a power law. In particular, seawater supplies such a possibility in the region of 400-500 nm if extremely bioproductive waters are not considered and the chlorophyll absorption peak at 440 nm does not come out of the background of dissolved organic matter absorption. With these specific initial wavelengths, the elastic and Raman lidar returns differ only in the backscattering coefficients. Because the Raman-backscattering coefficient is constant along the profile, the (elastic-to-Raman) ratio of these lidar returns directly produces the profile of the elastic-backscattering coefficient. This technique stays valid even under multiple-scattering conditions, which is of great importance for seawater sounding.

  6. Retrievals of Profiles of Fine And Coarse Aerosols Using Lidar And Radiometric Space Measurements

    NASA Technical Reports Server (NTRS)

    Kaufman, Yoram; Tanre, Didier; Leon, Jean-Francois; Pelon, Jacques; Lau, William K. M. (Technical Monitor)

    2002-01-01

    In couple of years we expect the launch of the CALIPSO lidar spaceborne mission designed to observe aerosols and clouds. CALIPSO will collect profiles of the lidar attenuated backscattering coefficients in two spectral wavelengths (0.53 and 1.06 microns). Observations are provided along the track of the satellite around the globe from pole to pole. The attenuated backscattering coefficients are sensitive to the vertical distribution of aerosol particles, their shape and size. However the information is insufficient to be mapped into unique aerosol physical properties and vertical distribution. Infinite number of physical solutions can reconstruct the same two wavelength backscattered profile measured from space. CALIPSO will fly in formation with the Aqua satellite and the MODIS spectro-radiometer on board. Spectral radiances measured by MODIS in six channels between 0.55 and 2.13 microns simultaneously with the CALIPSO observations can constrain the solutions and resolve this ambiguity, albeit under some assumptions. In this paper we describe the inversion method and apply it to aircraft lidar and MODIS data collected over a dust storm off the coast of West Africa during the SHADE experiment. It is shown that the product of the single scattering albedo, omega, and the phase function, P, for backscattering can be retrieved from the synergism between measurements avoiding a priori hypotheses required for inverting lidar measurements alone. The resultant value of (omega)P(180 deg.) = 0.016/sr are significantly different from what is expected using Mie theory, but are in good agreement with recent results obtained from lidar observations of dust episodes. The inversion is robust in the presence of noise of 10% and 20% in the lidar signal in the 0.53 and 1.06 pm channels respectively. Calibration errors of the lidar of 5 to 10% can cause an error in optical thickness of 20 to 40% respectively in the tested cases. The lidar calibration errors cause degradation in the

  7. Measurements of Stratospheric Pinatubo Aerosol Extinction Profiles by a Raman Lidar

    NASA Technical Reports Server (NTRS)

    Abo, Makoto; Nagasawa, Chikao

    1992-01-01

    The Raman lidar has been used for remote measurements of water vapor, ozone and atmospheric temperature in the lower troposphere because the Raman cross section is three orders smaller than the Rayleigh cross section. We estimated the extinction coefficients of the Pinatubo volcanic aerosol in the stratosphere using a Raman lidar. If the precise aerosol extinction coefficients are derived, the backscatter coefficient of a Mie scattering lidar will be more accurately estimated. The Raman lidar has performed to measure density profiles of some species using Raman scattering. Here we used a frequency-doubled Nd:YAG laser for transmitter and received nitrogen vibrational Q-branch Raman scattering signal. Ansmann et al. (1990) derived tropospherical aerosol extinction profiles with a Raman lidar. We think that this method can apply to dense stratospheric aerosols such as Pinatubo volcanic aerosols. As dense aerosols are now accumulated in the stratosphere by Pinatubo volcanic eruption, the error of Ramen lidar signal regarding the fluctuation of air density can be ignored.

  8. Raman Lidar Measurements of Aerosol Extinction and Backscattering. Report 2; Derivation of Aerosol Real Refractive Index, Single-Scattering Albedo, and Humidification Factor using Raman Lidar and Aircraft Size Distribution

    NASA Technical Reports Server (NTRS)

    Ferrare, R. A.; Melfi, S. H.; Whiteman, D. N.; Evans, K. D.; Poellot, M.; Kaufman, Y. J.

    1998-01-01

    Aerosol backscattering and extinction profiles measured by the NASA Goddard Space Flight Center Scanning Raman Lidar (SRL) during the remote cloud sensing (RCS) intensive operations period (IOP) at the Department of Energy Atmospheric Radiation Measurement (ARM) southern Great Plains (SGP) site during two nights in April 1994 are discussed. These profiles are shown to be consistent with the simultaneous aerosol size distribution measurements made by a PCASP (Passive Cavity Aerosol Spectrometer Probe) optical particle counter flown on the University of North Dakota Citation aircraft. We describe a technique which uses both lidar and PCASP measurements to derive the dependence of particle size on relative humidity, the aerosol real refractive index n, and estimate the effective single-scattering albedo Omega(sub 0). Values of n ranged between 1.4-1.5 (dry) and 1.37-1.47 (wet); Omega(sub 0) varied between 0.7 and 1.0. The single-scattering albedo derived from this technique is sensitive to the manner in which absorbing particles are represented in the aerosol mixture; representing the absorbing particles as an internal mixture rather than the external mixture assumed here results in generally higher values of Omega(sub 0). The lidar measurements indicate that the change in particle size with relative humidity as measured by the PCASP can be represented in the form discussed by Hattel with the exponent gamma = 0.3 + or - 0.05. The variations in aerosol optical and physical characteristics captured in the lidar and aircraft size distribution measurements are discussed in the context of the meteorological conditions observed during the experiment.

  9. Raman lidar measurements of aerosol extinction and backscattering 2. Derivation of aerosol real refractive index, single-scattering albedo, and humidification factor using Raman lidar and aircraft size distribution measurements

    SciTech Connect

    Ferrare, R.A.; Melfi, S.H.; Whiteman, D.N.; Kaufman, Y.J.; Evans, K.D.

    1998-08-01

    Aerosol backscattering and extinction profiles measured by the NASA Goddard Space Flight Center Scanning Raman Lidar (SRL) during the remote cloud sensing (RCS) intensive operations period (IOP) at the Department of Energy Atmospheric Radiation Measurement (ARM) southern Great Plains (SGP) site during two nights in April 1994 are discussed. These profiles are shown to be consistent with the simultaneous aerosol size distribution measurements made by a PCASP (Passive Cavity Aerosol Spectrometer Probe) optical particle counter flown on the University of North Dakota Citation aircraft. We describe a technique which uses both lidar and PCASP measurements to derive the dependence of particle size on relative humidity, the aerosol real refractive index {ital n}, and estimate the effective single-scattering albedo {omega}{sub 0}. Values of {ital n} ranged between 1.4{endash}1.5 (dry) and 1.37{endash}1.47 (wet); {omega}{sub 0} varied between 0.7 and 1.0. The single-scattering albedo derived from this technique is sensitive to the manner in which absorbing particles are represented in the aerosol mixture; representing the absorbing particles as an internal mixture rather than the external mixture assumed here results in generally higher values of {omega}{sub 0}. The lidar measurements indicate that the change in particle size with relative humidity as measured by the PCASP can be represented in the form discussed by {ital Hanel} [1976] with the exponent {gamma}=0.3{plus_minus}0.05. The variations in aerosol optical and physical characteristics captured in the lidar and aircraft size distribution measurements are discussed in the context of the meteorological conditions observed during the experiment. {copyright} 1998 American Geophysical Union

  10. Atmospheric Backscatter Profiles at 1572nm from Pulsed Lidar Measurments of CO2 Column Absorption from the 2011 ASCENDS Flight Campaign

    NASA Astrophysics Data System (ADS)

    Allan, G. R.; Riris, H.; Hasselbrack, W.; Sun, X.; Ramanathan, A.; Mao, J.; Abshire, J. B.

    2012-12-01

    We present height-resolved backscatter profiles from the NASA Goddard Space Flight Center's CO2 sounder lidar, rich in detail, which shows clear evidence of multiple backscatter layers, clouds, and aerosols allowing for the identification of the Planetary Boundary Layer (PBL). This data is recorded as a consequence of our pulsed lidar measurements of the CO2 column absorption. The CO2 Sounder is a pulsed lidar for active remote measurements of CO2 abundance from an airborne platform and is one candidate for the lidar on the NASA ASCENDS mission. The lidar uses a scanning, pulsed laser and fiber amplifier in a Master Oscillator Power Amplifier (MOPA) configuration to measure CO2 absorption at 1572.335 nm, lineshape, range to scattering surface and backscatter profiles. The laser is scanned across the absorption feature measuring at 30 discrete wavelengths/scan and ~300 scans/sec. The time-resolved return signal, with a temporal resolution of 8ns, is detected by a photon-counting PMT fiber coupled to a modified commercial, 2m focal length f10 Schmidt-Cassegrain telescope. The column density for CO2 is estimated from the differential optical depth (DOD) of the scanned absorption line using an integrated-path differential absorption (IPDA) technique and the optical path from the time of flight. A backscatter profile of the measured column is recorded for every pulse of every scan and integrated for 1 second. The backscatter profiles we will show are determined from the receivers photon counting record using a cross-correaltion technique (sliding inner product) with a vertical resolution of better than 300m, set by the 1μs pulse width from the MOPA. The range to the surface can be determined to a few meters. Major benefits of a pulsed technique using time-resolved detection to measure lineshape, is the unambiguous detection of the ground return, intervening clouds, aerosols and information on the vertical distribution of CO2. This technique can uniquely identify the

  11. Dust layer profiling using an aerosol dropsonde

    NASA Astrophysics Data System (ADS)

    Ulanowski, Zbigniew; Kaye, Paul Henry; Hirst, Edwin; Wieser, Andreas; Stanley, Warren

    2015-04-01

    Routine meteorological data is obtained in the atmosphere using disposable radiosondes, giving temperature, pressure, humidity and wind speed. Additional measurements are obtained from dropsondes, released from research aircraft. However, a crucial property not yet measured is the size and concentration of atmospheric particulates, including dust. Instead, indirect measurements are employed, relying on remote sensing, to meet the demands from areas such as climate research, air quality monitoring, civil emergencies etc. In addition, research aircraft can be used in situ, but airborne measurements are expensive, and aircraft use is restricted to near-horizontal profiling, which can be a limitation, as phenomena such as long-range transport depend on the vertical distribution of aerosol. The Centre for Atmospheric and Instrumentation Research at University of Hertfordshire develops light-scattering instruments for the characterization of aerosols and cloud particles. Recently a range of low-cost, miniature particle counters has been created, intended for use with systems such as disposable balloon-borne radiosondes, dropsondes, or in dense ground-based sensor networks. Versions for different particle size ranges exist. They have been used for vertical profiling of aerosols such as mineral dust or volcanic ash. A disadvantage of optical particle counters that sample through a narrow inlet is that they can become blocked, which can happen in cloud, for example. Hence, a different counter version has been developed, which can have open-path geometry, as the sensing zone is defined optically rather than being delimited by the flow system. This counter has been used for ground based air-quality monitoring around Heathrow airport. The counter has also been adapted for use with radiosondes or dropsondes. The dropsonde version has been successfully tested by launching it from research aircraft together with the so-called KITsonde, developed at the Karlsruhe Institute of

  12. Simulation of positron backscattering and implantation profiles using Geant4 code

    NASA Astrophysics Data System (ADS)

    Huang, Shi-Juan; Pan, Zi-Wen; Liu, Jian-Dang; Han, Rong-Dian; Ye, Bang-Jiao

    2015-10-01

    For the proper interpretation of the experimental data produced in slow positron beam technique, the positron implantation properties are studied carefully using the latest Geant4 code. The simulated backscattering coefficients, the implantation profiles, and the median implantation depths for mono-energetic positrons with energy range from 1 keV to 50 keV normally incident on different crystals are reported. Compared with the previous experimental results, our simulation backscattering coefficients are in reasonable agreement, and we think that the accuracy may be related to the structures of the host materials in the Geant4 code. Based on the reasonable simulated backscattering coefficients, the adjustable parameters of the implantation profiles which are dependent on materials and implantation energies are obtained. The most important point is that we calculate the positron backscattering coefficients and median implantation depths in amorphous polymers for the first time and our simulations are in fairly good agreement with the previous experimental results. Project supported by the National Natural Science Foundation of China (Grant Nos. 11175171 and 11105139).

  13. Vertically-resolved profiles of mass concentrations and particle backscatter coefficients of Asian dust plumes derived from lidar observations of silicon dioxide.

    PubMed

    Noh, Youngmin; Müller, Detlef; Shin, Sung-Kyun; Shin, Dongho; Kim, Young J

    2016-01-01

    This study presents a method to retrieve vertically-resolved profiles of dust mass concentrations by analyzing Raman lidar signals of silicon dioxide (quartz) at 546nm. The observed particle plumes consisted of mixtures of East Asian dust with anthropogenic pollution. Our method for the first time allows for extracting the contribution of the aerosol component "pure dust" contained in the aerosol type "polluted dust". We also propose a method that uses OPAC (Optical Properties of Aerosols and Clouds) and the mass concentrations profiles of dust in order to derive profiles of backscatter coefficients of pure dust in mixed dust/pollution plumes. The mass concentration of silicon dioxide (quartz) in the atmosphere can be estimated from the backscatter coefficient of quartz. The mass concentration of dust is estimated by the weight percentage (38-77%) of mineral quartz in Asian dust. The retrieved dust mass concentrations are classified into water soluble, nucleation, accumulation, mineral-transported and coarse mode according to OPAC. The mass mixing ratio of 0.018, 0.033, 0.747, 0.130 and 0.072, respectively, is used. Dust extinction coefficients at 550nm were calculated by using OPAC and prescribed number concentrations for each of the 5 components. Dust backscatter coefficients were calculated from the dust extinction coefficients on the basis of a lidar ratio of 45±3sr at 532nm. We present results of quartz-Raman measurements carried out on the campus of the Gwangju Institute of Science and Technology (35.10°N, 126.53°E) on 15, 16, and 21 March 2010.

  14. Systematic observations of long-range transport events and climatological backscatter profiles with the DWD ceilometer network

    NASA Astrophysics Data System (ADS)

    Mattis, Ina; Müller, Gerhard; Wagner, Frank; Hervo, Maxime

    2015-04-01

    about 6 days per station, the optical depth of the dust particles was estimated to be larger than 0.4. Those events are classified as 'strong'. 'Faint', 'weak', and 'medium' events were detected at 13, 15, and 12 days per station, respectively. Almost all of the forest fire events have been classified as 'faint' and 'weak' with optical depths below 0.15. Beside this qualitative investigations on transport events, we started to obtain calibration constants for all individual ceilometers in our network within the framework of the European projects E-PROFILE and TOPROF. We are currently producing a data set of 1-hour-mean particle backscatter profiles at 1064 nm at all ceilometer stations in Germany for the period between summer 2013 and winter 2014. We will present an overview on the used methodologies of analysis of long-range transport events and of the calibration procedures. More detailed results of the event analysis, e.g. on seasonal behaviour will be presented as well. Further we will show results of a first statistical analysis of our 18-months data set of backscatter profiles over Germany.

  15. Lidar Ratios for Dust Aerosols Derived From Retrievals of CALIPSO Visible Extinction Profiles Constrained by Optical Depths from MODIS-Aqua and CALIPSO/CloudSat Ocean Surface Reflectance Measurements

    NASA Technical Reports Server (NTRS)

    Young, Stuart A.; Josset, Damien B.; Vaughan, Mark A.

    2010-01-01

    CALIPSO's (Cloud Aerosol Lidar Infrared Pathfinder Satellite Observations) analysis algorithms generally require the use of tabulated values of the lidar ratio in order to retrieve aerosol extinction and optical depth from measured profiles of attenuated backscatter. However, for any given time or location, the lidar ratio for a given aerosol type can differ from the tabulated value. To gain some insight as to the extent of the variability, we here calculate the lidar ratio for dust aerosols using aerosol optical depth constraints from two sources. Daytime measurements are constrained using Level 2, Collection 5, 550-nm aerosol optical depth measurements made over the ocean by the MODIS (Moderate Resolution Imaging Spectroradiometer) on board the Aqua satellite, which flies in formation with CALIPSO. We also retrieve lidar ratios from night-time profiles constrained by aerosol column optical depths obtained by analysis of CALIPSO and CloudSat backscatter signals from the ocean surface.

  16. Characterization of Florida red tide aerosol and the temporal profile of aerosol concentration.

    PubMed

    Cheng, Yung Sung; Zhou, Yue; Pierce, Richard H; Henry, Mike; Baden, Daniel G

    2010-05-01

    Red tide aerosols containing aerosolized brevetoxins are produced during the red tide bloom and transported by wind to coastal areas of Florida. This study reports the characterization of Florida red tide aerosols in human volunteer studies, in which an asthma cohort spent 1h on Siesta Beach (Sarasota, Florida) during aerosolized red tide events and non-exposure periods. Aerosol concentrations, brevetoxin levels, and particle size distribution were measured. Hourly filter samples were taken and analyzed for brevetoxin and NaCl concentrations. In addition, the aerosol mass concentration was monitored in real time. The results indicated that during a non-exposure period in October 2004, no brevetoxin was detected in the water, resulting in non-detectable levels of brevetoxin in the aerosol. In March 2005, the time-averaged concentrations of brevetoxins in water samples were moderate, in the range of 5-10 microg/L, and the corresponding brevetoxin level of Florida red tide aerosol ranged between 21 and 39 ng/m(3). The temporal profiles of red tide aerosol concentration in terms of mass, NaCl, and brevetoxin were in good agreement, indicating that NaCl and brevetoxins are components of the red tide aerosol. By continuously monitoring the marine aerosol and wind direction at Siesta Beach, we observed that the marine aerosol concentration varied as the wind direction changed. The temporal profile of the Florida red tide aerosol during a sampling period could be explained generally with the variation of wind direction.

  17. Characterization of Florida red tide aerosol and the temporal profile of aerosol concentration

    PubMed Central

    Cheng, Yung Sung; Zhou, Yue; Pierce, Richard H.; Henry, Mike; Baden, Daniel G.

    2009-01-01

    Red tide aerosols containing aerosolized brevetoxins are produced during the red tide bloom and transported by wind to coastal areas of Florida. This study reports the characterization of Florida red tide aerosols in human volunteer studies, in which an asthma cohort spent 1 h on Siesta Beach (Sarasota, Florida) during aerosolized red tide events and non-exposure periods. Aerosol concentrations, brevetoxin levels, and particle size distribution were measured. Hourly filter samples were taken and analyzed for brevetoxin and NaCl concentrations. In addition, the aerosol mass concentration was monitored in real time. The results indicated that during a non-exposure period in October 2004, no brevetoxin was detected in the water, resulting in non-detectable levels of brevetoxin in the aerosol. In March 2005, the time-averaged concentrations of brevetoxins in water samples were moderate, in the range of 5–10 μg/L, and the corresponding brevetoxin level of Florida red tide aerosol ranged between 21 and 39 ng/m3. The temporal profiles of red tide aerosol concentration in terms of mass, NaCl, and brevetoxin were in good agreement, indicating that NaCl and brevetoxins are components of the red tide aerosol. By continuously monitoring the marine aerosol and wind direction at Siesta Beach, we observed that the marine aerosol concentration varied as the wind direction changed. The temporal profile of the Florida red tide aerosol during a sampling period could be explained generally with the variation of wind direction. PMID:19879288

  18. Studying the vertical aerosol extinction coefficient by comparing in situ airborne data and elastic backscatter lidar

    NASA Astrophysics Data System (ADS)

    Rosati, Bernadette; Herrmann, Erik; Bucci, Silvia; Fierli, Federico; Cairo, Francesco; Gysel, Martin; Tillmann, Ralf; Größ, Johannes; Gobbi, Gian Paolo; Di Liberto, Luca; Di Donfrancesco, Guido; Wiedensohler, Alfred; Weingartner, Ernest; Virtanen, Annele; Mentel, Thomas F.; Baltensperger, Urs

    2016-04-01

    Vertical profiles of aerosol particle optical properties were explored in a case study near the San Pietro Capofiume (SPC) ground station during the PEGASOS Po Valley campaign in the summer of 2012. A Zeppelin NT airship was employed to investigate the effect of the dynamics of the planetary boundary layer at altitudes between ˜ 50 and 800 m above ground. Determined properties included the aerosol particle size distribution, the hygroscopic growth factor, the effective index of refraction and the light absorption coefficient. The first three parameters were used to retrieve the light scattering coefficient. Simultaneously, direct measurements of both the scattering and absorption coefficient were carried out at the SPC ground station. Additionally, a single wavelength polarization diversity elastic lidar system provided estimates of aerosol extinction coefficients using the Klett method to accomplish the inversion of the signal, for a vertically resolved comparison between in situ and remote-sensing results. Note, however, that the comparison was for the most part done in the altitude range where the overlap function is incomplete and accordingly uncertainties are larger. First, the airborne results at low altitudes were validated with the ground measurements. Agreement within approximately ±25 and ±20 % was found for the dry scattering and absorption coefficient, respectively. The single scattering albedo, ranged between 0.83 and 0.95, indicating the importance of the absorbing particles in the Po Valley region. A clear layering of the atmosphere was observed during the beginning of the flight (until ˜ 10:00 LT - local time) before the mixing layer (ML) was fully developed. Highest extinction coefficients were found at low altitudes, in the new ML, while values in the residual layer, which could be probed at the beginning of the flight at elevated altitudes, were lower. At the end of the flight (after ˜ 12:00 LT) the ML was fully developed, resulting in

  19. Aerosol profiling by Raman lidar in Nanjing, China

    NASA Astrophysics Data System (ADS)

    Cao, Nianwen; Yang, Shaobo; Xie, Yinhai; Zhu, Cunxiong

    2015-10-01

    Aerosol profiles at 607 nm over ranges from 2 to 20 km were obtained using Raman lidar in Nanjing, China. The measured aerosol extinction coefficient was largely stable at about 1.5-2.5 × 10-4 m-1 after noise and Rayleigh corrections were applied. The noise effect in Raman lidar aerosol measurements is analyzed, and a formula relating aerosol extinction coefficient error and noise is presented in detail. Simulation and experimental results are in good agreement, indicating that the noise-related calculation for the Raman lidar aerosol measurement error is reasonable.

  20. The Cloud-Aerosol Transport System (CATS): A New Lidar for Aerosol and Cloud Profiling from the International Space Station

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth J.; McGill, Mathew J.; Yorks. John E.; Hlavka, Dennis L.; Hart, William D.; Palm, Stephen P.; Colarco, Peter R.

    2012-01-01

    Spaceborne lidar profiling of aerosol and cloud layers has been successfully implemented during a number of prior missions, including LITE, ICESat, and CALIPSO. Each successive mission has added increased capability and further expanded the role of these unique measurements in wide variety of applications ranging from climate, to air quality, to special event monitoring (ie, volcanic plumes). Many researchers have come to rely on the availability of profile data from CALIPSO, especially data coincident with measurements from other A-Train sensors. The CALIOP lidar on CALIPSO continues to operate well as it enters its fifth year of operations. However, active instruments have more limited lifetimes than their passive counterparts, and we are faced with a potential gap in lidar profiling from space if the CALIOP lidar fails before a new mission is operational. The ATLID lidar on EarthCARE is not expected to launch until 2015 or later, and the lidar component of NASA's proposed Aerosols, Clouds, and Ecosystems (ACE) mission would not be until after 2020. Here we present a new aerosol and cloud lidar that was recently selected to provide profiling data from the International Space Station (ISS) starting in 2013. The Cloud-Aerosol Transport System (CATS) is a three wavelength (1064,532,355 nm) elastic backscatter lidar with HSRL capability at 532 nm. Depolarization measurements will be made at all wavelengths. The primary objective of CATS is to continue the CALIPSO aerosol and cloud profile data record, ideally with overlap between both missions and EarthCARE. In addition, the near real time (NRT) data capability ofthe ISS will enable CATS to support operational applications such as aerosol and air quality forecasting and special event monitoring. The HSRL channel will provide a demonstration of technology and a data testbed for direct extinction retrievals in support of ACE mission development. An overview of the instrument and mission will be provided, along with a

  1. Technique for Obtaining Vertical Profiles of Backscattering and Extinction Cross Sections Using Slant Path Lidar Measurements

    NASA Technical Reports Server (NTRS)

    Spinhirne, J. D.; Herman, B. M.

    1973-01-01

    A method is presented for solving for vertical profiles of atmospheric particulate extinction and backscattering cross-sections utilizing monostatic lidar slant path measurements. The method is an extension of work by Fernald. It is shown that the number of assumptions necessary for an iterative solution of extinction and backscattering cross sections can be reduced if lidar slant path measurements are used to solve directly for optical depths. The technique is useful only if sufficiently accurate lidar measurements are available. With highly accurate measurements it is also possible to solve directly for extinction cross sections without an iterative solution of a transcendental equation if the proper reduction scheme is used. The required accuracy is discussed and results showing the effect of errors are presented.

  2. Comparison of MADE3-simulated and observed aerosol distributions with a focus on aerosol vertical profiles

    NASA Astrophysics Data System (ADS)

    Kaiser, Christopher; Hendricks, Johannes; Righi, Mattia; Jöckel, Patrick

    2016-04-01

    The reliability of aerosol radiative forcing estimates from climate models depends on the accuracy of simulated global aerosol distribution and composition, as well as on the models' representation of the aerosol-cloud and aerosol-radiation interactions. To help improve on previous modeling studies, we recently developed the new aerosol microphysics submodel MADE3 that explicitly tracks particle mixing state in the Aitken, accumulation, and coarse mode size ranges. We implemented MADE3 into the global atmospheric chemistry general circulation model EMAC and evaluated it by comparison of simulated aerosol properties to observations. Compared properties include continental near-surface aerosol component concentrations and size distributions, continental and marine aerosol vertical profiles, and nearly global aerosol optical depth. Recent studies have shown the specific importance of aerosol vertical profiles for determination of the aerosol radiative forcing. Therefore, our focus here is on the evaluation of simulated vertical profiles. The observational data is taken from campaigns between 1990 and 2011 over the Pacific Ocean, over North and South America, and over Europe. The datasets include black carbon and total aerosol mass mixing ratios, as well as aerosol particle number concentrations. Compared to other models, EMAC with MADE3 yields good agreement with the observations - despite a general high bias of the simulated mass mixing ratio profiles. However, BC concentrations are generally overestimated by many models in the upper troposphere. With MADE3 in EMAC, we find better agreement of the simulated BC profiles with HIPPO data than the multi-model average of the models that took part in the AeroCom project. There is an interesting difference between the profiles from individual campaigns and more "climatological" datasets. For instance, compared to spatially and temporally localized campaigns, the model simulates a more continuous decline in both total

  3. Demonstration of Aerosol Property Profiling by Multi-wavelength Lidar Under Varying Relative Humidity Conditions

    NASA Technical Reports Server (NTRS)

    Whiteman, D.N.; Veselovskii, I.; Kolgotin, A.; Korenskii, M.; Andrews, E.

    2008-01-01

    The feasibility of using a multi-wavelength Mie-Raman lidar based on a tripled Nd:YAG laser for profiling aerosol physical parameters in the planetary boundary layer (PBL) under varying conditions of relative humidity (RH) is studied. The lidar quantifies three aerosol backscattering and two extinction coefficients and from these optical data the particle parameters such as concentration, size and complex refractive index are retrieved through inversion with regularization. The column-integrated, lidar-derived parameters are compared with results from the AERONET sun photometer. The lidar and sun photometer agree well in the characterization of the fine mode parameters, however the lidar shows less sensitivity to coarse mode. The lidar results reveal a strong dependence of particle properties on RH. The height regions with enhanced RH are characterized by an increase of backscattering and extinction coefficient and a decrease in the Angstrom exponent coinciding with an increase in the particle size. We present data selection techniques useful for selecting cases that can support the calculation of hygroscopic growth parameters using lidar. Hygroscopic growth factors calculated using these techniques agree with expectations despite the lack of co-located radiosonde data. Despite this limitation, the results demonstrate the potential of multi-wavelength Raman lidar technique for study of aerosol humidification process.

  4. Development of ATLID-MSI synergy for retrieving the vertical profiles of aerosol components

    NASA Astrophysics Data System (ADS)

    Kudo, R.; Nishizawa, T.; Higurashi, A.; Sugimoto, N.; Oikawa, E.

    2014-12-01

    EarthCARE is an earth observation satellite and will be launched in 2016. Using its two sensors, ATLID (High spectral resolution lidar) and MSI (Multi-spectral imager), we are developing the synergy algorithm to retrieve the vertical profiles of extinction coefficients at 355 nm of four aerosol components (Water-soluble, black carbon, dust, and sea-salt particles), and the column mean of mode radii of water-soluble and dust particles. The ATLID data are extinction coefficient, backscatter coefficient, and depolarization ratio for total aerosols at 355 nm. The MSI data are radiances at 670 and 865 nm. The dry volume concentrations of four aerosol components at each altitude and the mode radii of water-soluble and dust particles in the column are simultaneously optimized to ATLID and MSI data by the gauss newton method. After the optimization, the vertical profiles of the extinction coefficient at 355 nm of four aerosol components are obtained. The size distributions of four aerosol components are assumed to be a lognormal distribution. The refractive indices of four aerosol components are given from previously observational studies. The humidity growth is considered for water-soluble and sea-salt particles. The volume concentration and the mode radius of the sea-salt particle are parameterized using the surface wind speed on the ocean. We assumed that the shape of the water-soluble, black carbon, and sea-salt particles are spherical, and the shape of the dust particle is spheroidal. We tested the algorithm using the ATLID and MSI data simulated using clean, dust-transported, and smoke-transported aerosols. The extinction coefficients of each component at 355 nm are retrieved well. The mode radius of water-soluble and dust particles were somehow overestimated.

  5. Lidar observations of stratospheric aerosol over Mauna Loa Observatory, 1974 - 1981

    NASA Astrophysics Data System (ADS)

    Deluisi, J.; Defoor, T.; Coulson, K.; Fernald, F.; Thorne, K.

    1984-08-01

    One hundred seventy-three lidar profiles obtained during the year 1974 to 1981, inclusively are presented. Backscattering ratios are displayed in graphical form for 1-km intervals. Aerosol backscattering cross section, Rayleigh backscattering cross section, backscattering ratio and integrated optical depth are tabulated, also for 1-km intervals. The data reduction computer program is included.

  6. Quasi-analytical determination of noise-induced error limits in lidar retrieval of aerosol backscatter coefficient by the elastic, two-component algorithm.

    PubMed

    Sicard, Michaël; Comerón, Adolfo; Rocadenbosch, Francisco; Rodríguez, Alejandro; Muñoz, Constantino

    2009-01-10

    The elastic, two-component algorithm is the most common inversion method for retrieving the aerosol backscatter coefficient from ground- or space-based backscatter lidar systems. A quasi-analytical formulation of the statistical error associated to the aerosol backscatter coefficient caused by the use of real, noise-corrupted lidar signals in the two-component algorithm is presented. The error expression depends on the signal-to-noise ratio along the inversion path and takes into account "instantaneous" effects, the effect of the signal-to-noise ratio at the range where the aerosol backscatter coefficient is being computed, as well as "memory" effects, namely, both the effect of the signal-to-noise ratio in the cell where the inversion is started and the cumulative effect of the noise between that cell and the actual cell where the aerosol backscatter coefficient is evaluated. An example is shown to illustrate how the "instantaneous" effect is reduced when averaging the noise-contaminated signal over a number of cells around the range where the inversion is started.

  7. Phase function, backscatter, extinction, and absorption for standard radiation atmosphere and El Chichon aerosol models at visible and near-infrared wavelengths

    NASA Technical Reports Server (NTRS)

    Whitlock, C. H.; Suttles, J. T.; Lecroy, S. R.

    1985-01-01

    Tabular values of phase function, Legendre polynominal coefficients, 180 deg backscatter, and extinction cross section are given for eight wavelengths in the atmospheric windows between 0.4 and 2.2 microns. Also included are single scattering albedo, asymmetry factor, and refractive indices. These values are based on Mie theory calculations for the standard rediation atmospheres (continental, maritime, urban, unperturbed stratospheric, volcanic, upper atmospheric, soot, oceanic, dust, and water-soluble) assest measured volcanic aerosols at several time intervals following the El Chichon eruption. Comparisons of extinction to 180 deg backscatter for different aerosol models are presented and related to lidar data.

  8. New approach for aerosol profiling with a lidar onboard an ultralight aircraft: application to the African Monsoon Multidisciplinary Analysis.

    PubMed

    Chazette, Patrick; Sanak, Joseph; Dulac, François

    2007-12-15

    A new airborne instrumental payload has been designed for an ultralight aircraft to determine the vertical profile of aerosol optical properties. It is based on Lidar Aérosols UltraViolet Aéroporté (LAUVA), a compact backscattering lidar system emitting at the wavelength of 355 nm. We operated this airborne configuration in the Sahel from the city of Niamey (Niger) during the first campaign of the African Monsoon Multidisciplinary Analysis (AMMA) in January-February 2006, when aerosols from both soil dust and savannah fires cause large visibility reductions. We take advantage of the lidar capability of pointing in different directions for retrieving the vertical profile of the aerosol backscatter to extinction ratio (BER). A synergy with a scatterometer (880 nm) and a ground-based sunphotometer allows us to further determine the vertical profile of Angström exponent (a). We identify three types of aerosol layers up to about 5 km below the free troposphere, dominated by biomass burning (BB) particles, mineral dust (D) particles, and a mixing between BB and D particles, respectively, associated with BER (a) values close to 0.008 sr(-1) (1.5), 0.025 sr(-1) (0), and 0.015 sr(-1) (0.4-1).

  9. Ceilometer for aerosol profiling: comparison with the multiwavelength in the frame of INTERACT (INTERcomparison of Aerosol and Cloud Tracking)

    NASA Astrophysics Data System (ADS)

    Madonna, Fabio; Vande Hey, Joshua; Rosoldi, Marco; Amato, Francesco; Pappalardo, Gelsomina

    2015-04-01

    project. This work is the first time that three different commercial ceilometers with an advanced Raman lidar are compared over a period of six months. The comparison of the attenuated backscatter profiles from a multi-wavelength Raman lidar and three ceilometers (CHM15k, CS135s, CT25K) reveals differences due to the expected discrepancy in the SNR but also due to effect of changes in the ambient temperature on the short and mid-term stability of ceilometer calibration. A large instability of ceilometers in the incomplete overlap region has also been observed, making the use of a single overlap correction function for the whole duration of the campaign critical. Therefore, technological improvements of ceilometers towards their operational use in the monitoring of the atmospheric aerosol in the low and free troposphere are needed.

  10. Aerosols and Precipitation Retrievals over Eureka by Remote Sensing: Validation of Space Based Profiling Retrievals

    NASA Astrophysics Data System (ADS)

    Chaubey, J. P.; O'Neill, N. T.; Hudak, D. R.; Rodriguez, P.; Ivanescu, L.; Eloranta, E.; Duck, T.

    2014-12-01

    Aerosols and precipitation are among the agents responsible for the ongoing changes in the Arctic climate and the hydrological cycle. The seasonal variations of Arctic aerosols (Arctic haze for e.g.) are linked to the transport efficiency as well as precipitation (wet) scavenging. Aside from affecting aerosol concentrations, precipitation is an important hydrological variable that affects the moisture budget of the atmosphere. Aerosols, in turn, influence the vertical distribution of clouds and this induces changes in the precipitation pattern. The spatial and temporal sparsity of precipitation measurements over the Arctic region means that satellite remote sensing techniques take on an importance that considerably exceeds their role south of the Arctic circle. Radar reflectivity and snow profiles from CloudSat (in support of cloud and precipitation analyses) and backscattering measurements from CALIOP (investigations of aerosol and small cloud particle properties) can be used to study Arctic winter clouds and precipitation and the role of aerosols in their formation. In this study we attempt to validate satellite-based profiling retrievals of precipitation parameters using AHSRL (Arctic High Spectral Resolution Lidar), CRL (CANDAC Raman Lidar) and MMCR (Milli-Meter Cloud Radar) profiles acquired at the PEARL high-Arctic site in Eureka (80 °N, 86 °W), Nunavut, Canada. As part of the process of validating the profiling retrievals we aspire to learn more about the mechanisms controlling aerosol, cloud and precipitation inter-dynamics. In addition, ground-based, high-frequency observations of precipitation will be used for characterizing precipitation totals as well as the conditional probability of the type of precipitation (rain or snow) and thus to help understand and validate comparable information extracted from the satellite retrievals. We also aim to characterize different particle types using AHSRL and CRL depolarization profiles, MMCR Doppler velocity

  11. Recent Improvements to CALIOP Level 3 Aerosol Profile Product for Global 3-D Aerosol Extinction Characterization

    NASA Astrophysics Data System (ADS)

    Tackett, J. L.; Getzewich, B. J.; Winker, D. M.; Vaughan, M. A.

    2015-12-01

    With nine years of retrievals, the CALIOP level 3 aerosol profile product provides an unprecedented synopsis of aerosol extinction in three dimensions and the potential to quantify changes in aerosol distributions over time. The CALIOP level 3 aerosol profile product, initially released as a beta product in 2011, reports monthly averages of quality-screened aerosol extinction profiles on a uniform latitude/longitude grid for different cloud-cover scenarios, called "sky conditions". This presentation demonstrates improvements to the second version of the product which will be released in September 2015. The largest improvements are the new sky condition definitions which parse the atmosphere into "cloud-free" views accessible to passive remote sensors, "all-sky" views accessible to active remote sensors and "cloudy-sky" views for opaque and transparent clouds which were previously inaccessible to passive remote sensors. Taken together, the new sky conditions comprehensively summarize CALIOP aerosol extinction profiles for a broad range of scientific queries. In addition to dust-only extinction profiles, the new version will include polluted-dust and smoke-only extinction averages. A new method is adopted for averaging dust-only extinction profiles to reduce high biases which exist in the beta version of the level 3 aerosol profile product. This presentation justifies the new averaging methodology and demonstrates vertical profiles of dust and smoke extinction over Africa during the biomass burning season. Another crucial advancement demonstrated in this presentation is a new approach for computing monthly mean aerosol optical depth which removes low biases reported in the beta version - a scenario unique to lidar datasets.

  12. Retrievals of atmospheric CO2 from simulated space-borne measurements of backscattered near-infrared sunlight: accounting for aerosol effects.

    PubMed

    Butz, André; Hasekamp, Otto P; Frankenberg, Christian; Aben, Ilse

    2009-06-20

    Retrievals of atmospheric carbon dioxide (CO2) from space-borne measurements of backscattered near-infrared sunlight are hampered by aerosol and cirrus cloud scattering effects. We propose a retrieval approach that allows for the retrieval of a few effective aerosol parameters simultaneously with the CO2 total column by parameterizing particle amount, height distribution, and microphysical properties. Two implementations of the proposed method covering different spectral bands are tested for an ensemble of simulated nadir observations for aerosol (and cirrus) loaded scenes over low- and mid-latitudinal land surfaces. The residual aerosol-induced CO(2) errors are mostly below 1% up to aerosol optical thickness 0.5. The proposed methods also perform convincing for scenes where cirrus clouds of optical thickness 0.1 overlay the aerosol.

  13. Stratospheric aerosol profile retrievals from SCIAMACHY limb-scatter observations

    NASA Astrophysics Data System (ADS)

    Ernst, Florian; Von Savigny, PD Christian; Rozanov, Alexei; Bovensmann, Heinrich; Brinkhoff, Lena; Burrows, John

    2012-07-01

    Stratospheric aerosol extinction profiles are retrieved from SCIAMACHY/Envisat limb-scatter observations in the visible and near-IR spectral range. The retrieval scheme is based on an optimal estimation approach in combination with the radiative transfer model SCIATRAN and employs normalized and paired limb-radiance profiles at 470 nm and 750 nm. This contribution provides an overview of the retrieval approach adopted and includes first results on stratospheric aerosol time series spanning the entire duration of the Envisat mission, i.e. from fall 2002 to the present. The time series display obvious signatures of the volcanic eruptions as well as strong pyroCb events that occurred during the period studied. Comparison of the stratospheric extinction profiles with co-located SAGE II aerosol extinction profiles yields agreement of the global mean profiles within 20% between 15 and 35 km altitude.

  14. Parameterization of cloud lidar backscattering profiles by means of asymmetrical Gaussians.

    PubMed

    Guasta, M D; Morandi, M; Stefanutti, L

    1995-06-20

    A fitting procedure for cloud lidar data processing is shown that is based on the computation of the first three moments of the vertical-backscattering (or -extinction) profile. Single-peak clouds or single cloud layers are approximated to asymmetrical Gaussians. The algorithm is particularly stable with respect to noise and processing errors, and it is much faster than the equivalent least-squares approach. Multilayer clouds can easily be treated as a sum of single asymmetrical Gaussian peaks. The method is suitable for cloud-shape parametrization in noisy lidar signatures (like those expected from satellite lidars). It also permits an improvement of cloud radiative-property computations that are based on huge lidar data sets for which storage and careful examination of single lidar profiles can't be carried out.

  15. Profiling Transboundary Aerosols over Taiwan and Assessing Their Radiative Effects

    NASA Technical Reports Server (NTRS)

    Wang, Sheng-Hsiang; Lin, Neng-Huei; Chou, Ming-Dah; Tsay, Si-Chee; Welton, Ellsworth J.; Hsu, N. Christina; Giles, David M.; Liu, Gin-Rong; Holben, Brent N.

    2010-01-01

    A synergistic process was developed to study the vertical distributions of aerosol optical properties and their effects on solar heating using data retrieved from ground-based radiation measurements and radiative transfer simulations. Continuous MPLNET and AERONET observations were made at a rural site in northern Taiwan from 2005 to 2007. The aerosol vertical extinction profiles retrieved from ground-based lidar measurements were categorized into near-surface, mixed, and two-layer transport types, representing 76% of all cases. Fine-mode (Angstrom exponent, alpha, approx.1.4) and moderate-absorbing aerosols (columnar single-scattering albedo approx.0.93, asymmetry factor approx.0.73 at 440 nm wavelength) dominated in this region. The column-integrated aerosol optical thickness at 500 nm (tau(sub 500nm)) ranges from 0.1 to 0.6 for the near-surface transport type, but can be doubled in the presence of upper-layer aerosol transport. We utilize aerosol radiative efficiency (ARE; the impact on solar radiation per unit change of tau(sub 500nm)) to quantify the radiative effects due to different vertical distributions of aerosols. Our results show that the ARE at the top-of-atmosphere (-23 W/ sq m) is weakly sensitive to aerosol vertical distributions confined in the lower troposphere. On the other hand, values of the ARE at the surface are -44.3, -40.6 and -39.7 W/sq m 38 for near-surface, mixed, and two-layer transport types, respectively. Further analyses show that the impact of aerosols on the vertical profile of solar heating is larger for the near-surface transport type than that of two-layer transport type. The impacts of aerosol on the surface radiation and the solar heating profiles have implications for the stability and convection in the lower troposphere.

  16. A Lidar and Backscatter Sonde Aerosol Measurement Campaign at Table Mountain During February-March 1997: Observations of Stratospheric Background Aerosols and Cirrus Clouds

    NASA Technical Reports Server (NTRS)

    Beyerle, G.; Gross, M.; Haner, D.; Kjome, N.; McDermid, I.; McGee, T.; Rosen, J.; Schafer, H. J.; Schrems, O.

    1999-01-01

    Altitude profiles of backscater ratio of the stratospheric background aerosol layer at altitudes between 15 and 25 km and high-altitude cirrus clouds at altitudes below 13 km are analyzed and discussed. Cirrus clouds were present on 16 of the 26 campaign nights.

  17. Research on aerosol profiles and parameterization scheme in Southeast China

    NASA Astrophysics Data System (ADS)

    Wang, Gang; Deng, Tao; Tan, Haobo; Liu, Xiantong; Yang, Honglong

    2016-09-01

    The vertical distribution of the aerosol extinction coefficient serves as a basis for evaluating aerosol radiative forcing and air quality modeling. In this study, MODIS AOD data and ground-based lidar extinction coefficients were employed to verify 6 years (2009-2014) aerosol extinction data obtained via CALIOP for Southeast China. The objective was mainly to provide the parameterization scheme of annual and seasonal aerosol extinction profiles. The results showed that the horizontal and vertical distributions of CALIOP extinction data were highly accurate in Southeast China. The annual average AOD below 2 km accounted for 64% of the total layer, with larger proportions observed in winter (80%) and autumn (80%) and lower proportions observed in summer (70%) and spring (59%). The AOD was maximum in the spring (0.58), followed by the autumn and winter (0.44), and reached a minimum in the summer (0.40). The near-surface extinction coefficient increased from summer, spring, autumn and winter, in that order. The Elterman profile is obviously lower than the profiles observed by CALIOP in Southeast China. The annual average and seasonal aerosol profiles showed an exponential distribution, and could be divided into two sections. Two sections exponential fitting was used in the parameterization scheme. In the first section, the aerosol scale height reached 2200 m with a maximum (3,500 m) in summer and a minimum (1,230 m) in winter, which meant that the aerosol extinction decrease with height slower in summer, but more rapidly in winter. In second section, the aerosol scale height was maximum in spring, which meant that the higher aerosol diffused in spring.

  18. Implementation of Rotational Raman Channel in Multiwavelength Aerosol Lidar to Improve Measurements of Particle Extinction and Backscattering at 532 NM

    NASA Astrophysics Data System (ADS)

    Veselovskii, Igor; Whiteman, David N.; Korenskiy, Michael; Suvorina, A.; Perez-Ramirez, Daniel

    2016-06-01

    We describe a practical implementation of rotational Raman (RR) measurements in an existing Mie-Raman lidar to obtain measurements of aerosol extinction and backscattering at 532 nm. A 2.3 nm width interference filter was used to select a spectral range characterized by low temperature sensitivity within the anti-Stokes branch of the RR spectrum. Simulations demonstrate that the temperature dependence of the scattering cross section does not exceed 1.0% in the 230-300K range making accurate correction for this dependence quite easy. With this upgrade, the NASA/GSFC multiwavelength Raman lidar has demonstrated useful α532 measurements and was used for regular observations. Examples of lidar measurements and inversion of optical data to the particle microphysics will be given in presentation.

  19. Ceilometer Aerosol Profiling versus Raman Lidar in the Frame of Interact Campaign of Actris

    NASA Astrophysics Data System (ADS)

    Madonna, F.; Amato, F.; Rosoldi, M.; Vande Hey, J.; Pappalardo, G.

    2016-06-01

    In this paper, multi-wavelength Raman lidar measurements are used to investigate the capability of ceilometers to provide reliable information about atmospheric aerosol properties through the INTERACT (INTERcomparison of Aerosol and Cloud Tracking) campaign carried out at the CNR-IMAA Atmospheric Observatory (760 m a.s.l., 40.60 N, 15.72 E), in the framework of ACTRIS (Aerosol Clouds Trace gases Research InfraStructure) FP7 project. This work is the first time that three different commercial ceilometers with an advanced Raman lidar are compared over a period of six month. The comparison of the attenuated backscatter coefficient profiles from a multi-wavelength Raman lidar and three ceilometers (CHM15k, CS135s, CT25K) reveals differences due to the expected discrepancy in the SNR but also due to effect of changes in the ambient temperature on the stability of ceilometer calibration over short and mid-term. Technological improvements of ceilometers towards their operational use in the monitoring of the atmospheric aerosol in the low and free troposphere are likely needed.

  20. Ceilometer aerosol profiling versus Raman lidar in the frame of the INTERACT campaign of ACTRIS

    NASA Astrophysics Data System (ADS)

    Madonna, F.; Amato, F.; Vande Hey, J.; Pappalardo, G.

    2015-05-01

    Despite their differences from more advanced and more powerful lidars, the low construction and operation cost of ceilometers (originally designed for cloud base height monitoring) has fostered their use for the quantitative study of aerosol properties. The large number of ceilometers available worldwide represents a strong motivation to investigate both the extent to which they can be used to fill in the geographical gaps between advanced lidar stations and also how their continuous data flow can be linked to existing networks of the more advanced lidars, like EARLINET (European Aerosol Research Lidar Network). In this paper, multi-wavelength Raman lidar measurements are used to investigate the capability of ceilometers to provide reliable information about atmospheric aerosol properties through the INTERACT (INTERcomparison of Aerosol and Cloud Tracking) campaign carried out at the CNR-IMAA Atmospheric Observatory (760 m a.s.l., 40.60° N, 15.72° E), in the framework of the ACTRIS (Aerosol Clouds Trace gases Research InfraStructure) FP7 project. This work is the first time that three different commercial ceilometers with an advanced Raman lidar are compared over a period of 6 months. The comparison of the attenuated backscatter coefficient profiles from a multi-wavelength Raman lidar and three ceilometers (CHM15k, CS135s, CT25K) reveals differences due to the expected discrepancy in the signal to noise ratio (SNR) but also due to changes in the ambient temperature on the short and mid-term stability of ceilometer calibration. Therefore, technological improvements are needed to move ceilometers towards operational use in the monitoring of atmospheric aerosols in the low and free troposphere.

  1. Ceilometer aerosol profiling vs. Raman lidar in the frame of INTERACT campaign of ACTRIS

    NASA Astrophysics Data System (ADS)

    Madonna, F.; Amato, F.; Vande Hey, J.; Pappalardo, G.

    2014-12-01

    Despite their differences from more advanced and more powerful lidars, the low construction and operation cost of ceilometers, originally designed for cloud base height monitoring, has fostered their use for the quantitative study of aerosol properties. The large number of ceilometers available worldwide represents a strong motivation to investigate both the extent to which they can be used to fill in the geographical gaps between advanced lidar stations and also how their continuous data flow can be linked to existing networks of the more advanced lidars, like EARLINET (European Aerosol Research LIdar NETwork). In this paper, multi-wavelength Raman lidar measurements are used to investigate the capability of ceilometers to provide reliable information about atmospheric aerosol content through the INTERACT (INTERcomparison of Aerosol and Cloud Tracking) campaign carried out at the CNR-IMAA Atmospheric Observatory (760 m a.s.l., 40.60° N, 15.72° E), in the framework of ACTRIS (Aerosol Clouds Trace gases Research InfraStructure) FP7 project. This work is the first time that three different commercial ceilometers with an advanced Raman lidar are compared over a period of six months. The comparison of the attenuated backscatter profiles from a multi-wavelength Raman lidar and three ceilometers (CHM15k, CS135s, CT25K) reveals differences due to the expected discrepancy in the SNR but also due to effect of changes in the ambient temperature on the short and mid-term stability of ceilometer calibration. A large instability of ceilometers in the incomplete overlap region has also been observed, making the use of a single overlap correction function for the whole duration of the campaign critical. Therefore, technological improvements of ceilometers towards their operational use in the monitoring of the atmospheric aerosol in the low and free troposphere are needed.

  2. Determination of the particulate extinction-coefficient profile and the column-integrated lidar ratios using the backscatter-coefficient and optical-depth profiles.

    PubMed

    Kovalev, Vladimir A; Hao, Wei Min; Wold, Cyle

    2007-12-20

    A new method is considered that can be used for inverting data obtained from a combined elastic-inelastic lidar or a high spectral resolution lidar operating in a one-directional mode, or an elastic lidar operating in a multiangle mode. The particulate extinction coefficient is retrieved from the simultaneously measured profiles of the particulate backscatter coefficient and the particulate optical depth. The stepwise profile of the column-integrated lidar ratio is found that provides best matching of the initial (inverted) profile of the optical depth to that obtained by the inversion of the backscatter-coefficient profile. The retrieval of the extinction coefficient is made without using numerical differentiation. The method reduces the level of random noise in the retrieved extinction coefficient to the level of noise in the inverted backscatter coefficient. Examples of simulated and experimental data are presented.

  3. Tropospheric Vertical Profiles of Aerosol Optical, Microphysical and Concentration Properties in the Frame of the Hygra-CD Campaign (Athens, Greece 2014): A Case Study of Long-Range Transport of Mixed Aerosols

    NASA Astrophysics Data System (ADS)

    Papayannis, Alexandros; Argyrouli, Athina; Müller, Detlef; Tsaknakis, Georgios; Kokkalis, Panayotis; Binietoglou, Ioannis; Kazadzis, Stelios; Solomos, Stavros; Amiridis, Vassilis

    2016-06-01

    Combined multi-wavelength aerosol Raman lidar and sun photometry measurements were performed during the HYGRA-CD campaign over Athens, Greece during May-June 2014. The retrieved aerosol optical properties (3 aerosol backscatter at 355-532-1064 nm and 2 aerosol extinction profiles at 355-532 nm) were used as input to an inversion code to retrieve the aerosol microphysical properties (effective radius reff and number concentration N) using regularization techniques. Additionally, the volume concentration profile was derived for fine particles using the LIRIC code. In this paper we selected a complex case study of long-range transport of mixed aerosols (biomass burning particles mixed with dust) arriving over Athens between 10-12 June 2014 in the 1.5-4 km height. Between 2-3 km height we measured mean lidar ratios (LR) ranging from 45 to 58 sr (at 355 and 532 nm), while the Ångström exponent (AE) aerosol extinction-related values (355nm/532nm) ranged between 0.8-1.3. The retrieved values of reff and N ranged from 0.19±0.07 to 0.22±0.07 μm and 460±230 to 2200±2800 cm-3, respectively. The aerosol linear depolarization ratio (δ) at 532 nm was lower than 5-7% (except for the Saharan dust cases, where δ~10-15%).

  4. Near-surface fault detection by migrating back-scattered surface waves with and without velocity profiles

    NASA Astrophysics Data System (ADS)

    Yu, Han; Huang, Yunsong; Guo, Bowen

    2016-07-01

    We demonstrate that diffraction stack migration can be used to discover the distribution of near-surface faults. The methodology is based on the assumption that near-surface faults generate detectable back-scattered surface waves from impinging surface waves. We first isolate the back-scattered surface waves by muting or FK filtering, and then migrate them by diffraction migration using the surface wave velocity as the migration velocity. Instead of summing events along trial quasi-hyperbolas, surface wave migration sums events along trial quasi-linear trajectories that correspond to the moveout of back-scattered surface waves. We have also proposed a natural migration method that utilizes the intrinsic traveltime property of the direct and the back-scattered waves at faults. For the synthetic data sets and the land data collected in Aqaba, where surface wave velocity has unexpected perturbations, we migrate the back-scattered surface waves with both predicted velocity profiles and natural Green's function without velocity information. Because the latter approach avoids the need for an accurate velocity model in event summation, both the prestack and stacked migration images show competitive quality. Results with both synthetic data and field records validate the feasibility of this method. We believe applying this method to global or passive seismic data can open new opportunities in unveiling tectonic features.

  5. Profiling structured beams using injected aerosols

    NASA Astrophysics Data System (ADS)

    Loh, N. D.; Starodub, Dmitri; Lomb, Lukas; Hampton, Christina Y.; Martin, Andrew V.; Sierra, Raymond G.; Barty, Anton; Aquila, Andrew; Schulz, Joachim; Steinbrener, Jan; Shoeman, Robert L.; Kassemeyer, Stephan; Bostedt, Christoph; Bozek, John; Epp, Sascha W.; Erk, Benjamin; Hartmann, Robert; Rolles, Daniel; Rudenko, Artem; Rudek, Benedikt; Foucar, Lutz; Kimmel, Nils; Weidenspointner, Georg; Hauser, Günther; Holl, Peter; Pedersoli, Emanuele; Liang, MengNing; Hunter, Mark S.; Gumprecht, Lars; Coppola, Nicola; Wunderer, Cornelia; Graafsman, Heinz; Maia, Filipe R. N. C.; Ekeberg, Tomas; Hantke, Max; Fleckenstein, Holger; Hirsemann, Helmut; Nass, Karol; White, Thomas A.; Tobias, Herbert J.; Farquar, George R.; Benner, W. Henry; Hau-Riege, Stefan; Reich, Christian; Hartmann, Andreas; Soltau, Heike; Marchesini, Stefano; Bajt, Sasa; Barthelmess, Miriam; Strueder, Lothar; Ullrich, Joachim; Bucksbaum, Philip; Hodgson, Keith O.; Frank, Mathias; Schlichting, Ilme; Chapman, Henry N.; Bogan, Michael J.

    2012-10-01

    Profiling structured beams produced by X-ray free-electron lasers (FELs) is crucial to both maximizing signal intensity for weakly scattering targets and interpreting their scattering patterns. Earlier ablative imprint studies describe how to infer the X-ray beam profile from the damage that an attenuated beam inflicts on a substrate. However, the beams in-situ profile is not directly accessible with imprint studies because the damage profile could be different from the actual beam profile. On the other hand, although a Shack-Hartmann sensor is capable of in-situ profiling, its lenses may be quickly damaged at the intense focus of hard X-ray FEL beams. We describe a new approach that probes the in-situ morphology of the intense FEL focus. By studying the translations in diffraction patterns from an ensemble of randomly injected sub-micron latex spheres, we were able to determine the non-Gaussian nature of the intense FEL beam at the Linac Coherent Light Source (SLAC National Laboratory) near the FEL focus. We discuss an experimental application of such a beam-profiling technique, and the limitations we need to overcome before it can be widely applied.

  6. Global profiles of the direct aerosol effect using vertically resolved aerosol data

    NASA Astrophysics Data System (ADS)

    Korras Carraca, Marios Bruno; Pappas, Vasilios; Matsoukas, Christos; Hatzianastassiou, Nikolaos; Vardavas, Ilias

    2014-05-01

    Atmospheric aerosols, both natural and anthropogenic, can cause climate change through their direct, indirect, and semi-direct effects on the radiative energy budget of the Earth-atmosphere system. In general, aerosols cause cooling of the surface and the planet, while they warm the atmosphere due to scattering and absorption of incoming solar radiation. The importance of vertically resolved direct radiative effect (DRE) and heating/cooling effects of aerosols is strong, while large uncertainties still lie with their magnitudes. In order to be able to quantify them throughout the atmosphere, a detailed vertical profile of the aerosol effect is required. Such data were made available recently by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on board the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite. CALIOP is the first polarization lidar to fly in space and has been acquiring unique data on aerosols and clouds since June 2006. The aim of this study is to investigate both the vertically resolved geographic and seasonal variation of the DRE due to aerosols. The vertical profile of DRE under all-sky and clear-sky conditions is computed using the deterministic spectral radiative transfer model FORTH. From the DRE, the effect on atmospheric heating/cooling rate profiles due to aerosols can also be derived. We use CALIOP Level 2-Version 3 Layer aerosol optical depth data as input to our radiation transfer model, for a period of 3 complete years (2007-2009). These data are provided on a 5 km horizontal resolution and in up to 8 vertical layers and have been regridded on our model horizontal and vertical resolutions. We use cloud data from the International Satellite Cloud Climatology Project (ISCCP), while the aerosol asymmetry factor and single scattering albedo are taken from the Global Aerosol Data Set (GADS). The model computations are performed on a monthly, 2.5°× 2.5° resolution on global scale, at 40

  7. How well can we Measure the Vertical Profile of Tropospheric Aerosol Extinction?

    NASA Technical Reports Server (NTRS)

    Schmid, Beat; Ferrare, R.; Flynn, C.; Elleman, R.; Covert, D.; Strawa, A.; Welton, E.; Turner, D.; Jonsson, H.; Redemann, J.

    2005-01-01

    The recent Department of Energy Atmospheric Radiation Measurement (ARM) Aerosol Intensive Operations Period (MOP, May 2003) yielded one of the best measurement sets obtained to-date to assess our ability to measure the vertical profile of ambient aerosol extinction sigma(sub ep)(lambda) in the lower troposphere. During one month, a heavily instrumented aircraft with well characterized aerosol sampling ability carrying well proven and new aerosol instrumentation, devoted most of the 60 available flight hours to flying vertical profiles over the heavily instrumented ARM Southern Great Plains (SGP) Climate Research Facility (CRF). This allowed us to compare vertical extinction profiles obtained from 6 different instuments: airborne Sun photometer (AATS-14), airborne nephelometer/absorption photometer, airborne cavity ring-down system, ground-based Raman lidar and 2 ground-based elastic backscatter lidars. We find the in-situ measured sigma(sub ep)(lambda) to be lower than the AATS-14 derived values. Bias differences are 0.002 - 0.004 K/m equivalent to 12-17% in the visible, or 45% in the near-infrared. On the other hand, we find that with respect to AATS-14, the lidar sigma(sub ep)(lambda) are higher. An unnoticed loss of sensitivity of the Raman lidar had occurred leading up to AIOP and we expect better agreement from the recently restored system looking at the collective results from 6 field campaigns conducted since 1996, airborne in situ measurements of sigma(sub ep)(lambda) tend to be biased slightly low (17% at visible wavelengths) when compared to airborne Sun photometer sigma(sub ep)(lambda). On the other hand, sigma(sub ep)(lambda) values derived from lidars tend to have no or positive biases. From the bias differences we conclude that the typical systematic error associated with measuring the tropospheric vertical profile of the ambient aerosol extinction with current state of-the art instrumentation is 15-20% at visible wavelengths and potentially larger in

  8. ACTRIS aerosol vertical profile data and observations: potentiality and first examples of integrated studies with models

    NASA Astrophysics Data System (ADS)

    Mona, Lucia; Benedetti, Angela; D'Amico, Giuseppe; Myhre, Cathrine Lund; Schulz, Michael; Wandinger, Ulla; Laj, Paolo; Pappalardo, Gelsomina

    2016-04-01

    The ACTRIS-2 project, funded by Horizon 2020, addresses the scope of integrating state-of-the-art European ground-based stations for long term observations of aerosols, clouds and short lived gases, capitalizing on the work of FP7-ACTRIS. It aims at achieving the construction of a user-oriented RI, unique in the EU-RI landscape for providing 4-D integrated high-quality data from near-surface to high altitude (vertical profiles and total-column) which are relevant to climate and air-quality research. ACTRIS-2 develops and implements, in a large network of stations in Europe and beyond, observational protocols that permit the harmonization of collected data and their dissemination. ACTRIS secures provision and dissemination of a unique set of data and data-products that would not otherwise be available with the same level of quality and standardization. This results from a 10-year plus effort in constructing a research infrastructure capable of responding to community needs and requirements, and has been engaged since the start of the FP5 EU commission program. ACTRIS ensures compliance with reporting requirements (timing, format, traceability) defined by the major global observing networks. EARLINET (European Aerosol research Lidar NETwork), the aerosol vertical profiling component of ACTRIS, is providing since May 2000 vertical profiles of aerosol extinction and backscatter over Europe. A new structure of the EARLINET database has been designed in a more user oriented approach reporting new data products which are more effective for specific uses of different communities. In particular, a new era is starting with the Copernicus program during which the aerosol vertical profiling capability will be fundamental for assimilation and validation purposes. The new data products have been designed thanks to a strong link with EARLINET data users, first of all modeling and satellite communities, established since the beginning of EARLINET and re-enforced within ACTRIS2

  9. Profiling measurements of metal ion distribution in thin polymer inclusion membranes by Rutherford backscattering spectrometry

    NASA Astrophysics Data System (ADS)

    Guedioura, B.; Bendjaballah, N.; Alioui, N.

    2014-05-01

    Polymer inclusion membranes (PIMs) composed of a homogeneous mixture of cellulose triacetate matrix, 2-nitro-phenyl-octyl-ether as plasticizer and tri-octyl-phosphine-oxyde as carrier were synthesized by the spin coating method. Synthesized membranes were doped with molybdenum metal ions and then characterized by four experimental techniques: thermo gravimetric and differential analyses, scanning electron microscopy (SEM), attenuated total reflectance Fourier transform infrared (ATR-FTIR) spectroscopy and Rutherford backscattering (RBS) spectrometry using a 3.2 MeV He+ ion beam. The RBS analysis has established both the elemental composition as well as the Mo+ metal profiling of the studied PIMs. The experimental irradiation conditions were optimized in order to determine the ion fluence thresholds resulting in measurable changes in elemental composition of membranes. Changes in physico-chemical properties of the irradiated PIMs vs He+ ion fluence were observed with the ATR-FTIR analysis. Also, the SEM analysis of PIMs surfaces has revealed a porous texture, while the thermal analysis of annealed PIMs at 105°C has showed no significant changes of mass (∼1%) of the studied samples.

  10. In Situ Aerosol Profile Measurements and Comparisons with SAGE 3 Aerosol Extinction and Surface Area Profiles at 68 deg North

    NASA Technical Reports Server (NTRS)

    2005-01-01

    Under funding from this proposal three in situ profile measurements of stratospheric sulfate aerosol and ozone were completed from balloon-borne platforms. The measured quantities are aerosol size resolved number concentration and ozone. The one derived product is aerosol size distribution, from which aerosol moments, such as surface area, volume, and extinction can be calculated for comparison with SAGE III measurements and SAGE III derived products, such as surface area. The analysis of these profiles and comparison with SAGE III extinction measurements and SAGE III derived surface areas are provided in Yongxiao (2005), which comprised the research thesis component of Mr. Jian Yongxiao's M.S. degree in Atmospheric Science at the University of Wyoming. In addition analysis continues on using principal component analysis (PCA) to derive aerosol surface area from the 9 wavelength extinction measurements available from SAGE III. Ths paper will present PCA components to calculate surface area from SAGE III measurements and compare these derived surface areas with those available directly from in situ size distribution measurements, as well as surface areas which would be derived from PCA and Thomason's algorithm applied to the four wavelength SAGE II extinction measurements.

  11. Atmospheric aerosol profiling with a bistatic imaging lidar system.

    PubMed

    Barnes, John E; Sharma, N C Parikh; Kaplan, Trevor B

    2007-05-20

    Atmospheric aerosols have been profiled using a simple, imaging, bistatic lidar system. A vertical laser beam is imaged onto a charge-coupled-device camera from the ground to the zenith with a wide-angle lens (CLidar). The altitudes are derived geometrically from the position of the camera and laser with submeter resolution near the ground. The system requires no overlap correction needed in monostatic lidar systems and needs a much smaller dynamic range. Nighttime measurements of both molecular and aerosol scattering were made at Mauna Loa Observatory. The CLidar aerosol total scatter compares very well with a nephelometer measuring at 10 m above the ground. The results build on earlier work that compared purely molecular scattered light to theory, and detail instrument improvements. PMID:17514239

  12. Application of neural networks for determining optical parameters of strongly scattering media from the intensity profile of backscattered radiation

    SciTech Connect

    Kotova, S P; Maiorov, I V; Maiorova, A M

    2007-01-31

    We analyse the possibilities of simultaneous measuring three optical parameters of scattering media, namely, the scattering and absorption coefficients and the scattering anisotropy parameter by the intensity profile of backscattered radiation by using the neural network inversion method and the method of adaptive-network-based fuzzy inference system. The measurement errors of the absorption and scattering coefficients and the scattering anisotropy parameter are 20%, 5%, and 10%, respectively. (special issue devoted to multiple radiation scattering in random media)

  13. Vertical Profiles of Aerosol Optical and Microphysical Properties During a Rare Case of Long-range Transport of Mixed Biomass Burning-polluted Dust Aerosols from the Russian Federation-kazakhstan to Athens, Greece

    NASA Astrophysics Data System (ADS)

    Papayannis, Alexandros; Argyrouli, Athina; Kokkalis, Panayotis; Tsaknakis, Georgios; Binietoglou, Ioannis; Solomos, Stavros; Kazadzis, Stylianos; Samaras, Stefanos; Böckmann, Christine; Raptis, Panagiotis; Amiridis, Vassilis

    2016-06-01

    Multi-wavelength aerosol Raman lidar measurements with elastic depolarization at 532 nm were combined with sun photometry during the HYGRA-CD campaign over Athens, Greece, on May-June 2014. We retrieved the aerosol optical [3 aerosol backscatter profiles (baer) at 355-532-1064 nm, 2 aerosol extinction (aaer) profiles at 355-532 nm and the aerosol linear depolarization ratio (δ) at 532 nm] and microphysical properties [effective radius (reff), complex refractive index (m), single scattering albedo (ω)]. We present a case study of a long distance transport (~3.500-4.000 km) of biomass burning particles mixed with dust from the Russian Federation-Kazakhstan regions arriving over Athens on 21-23 May 2014 (1.7-3.5 km height). On 23 May, between 2-2.75 km we measured mean lidar ratios (LR) of 35 sr (355 nm) and 42 sr (532 nm), while the mean Ångström exponent (AE) aerosol backscatter-related values (355nm/532nm and 532nm/1064nm) were 2.05 and 1.22, respectively; the mean value of δ at 532 nm was measured to be 9%. For that day the retrieved mean aerosol microphysical properties at 2-2.75 km height were: reff=0.26 μm (fine mode), reff=2.15 μm (coarse mode), m=1.36+0.00024i, ω=0.999 (355 nm, fine mode), ω=0.992(355 nm, coarse mode), ω=0.997 (532 nm, fine mode), and ω=0.980 (532 nm, coarse mode).

  14. Lidar Aerosol Profiles Measured From Halifax During Summer 2007

    NASA Astrophysics Data System (ADS)

    Crawford, L.; Duck, T. J.; Doyle, J.; Harris, R.; Beauchamp, S.

    2007-12-01

    Measurements of aerosol profiles in the troposphere and lower stratosphere were obtained with a high-power Raman Lidar from Halifax, Nova Scotia (44.63N, 63.58W) on the East Coast of Canada during Summer 2007. Observations throughout the troposphere at high temporal resolution were made possible by using a new dual-receiver setup. The lidar was operated in clear-sky conditions, and several long duration (> 80 hours) data sets were obtained. The measurements reveal the presence of boundary-layer aerosols during episodes of pollution transport from the Eastern US and Canada, and are compared with surface measurements of ozone and other species. Boundary layer development, entrainment and mixing are evident in the data. Structured plumes at higher altitudes are traced back to biomass burning events throughout North America. Aerosols were also observed on two occasions at 15 km in altitude, and are most likely due to pyroconvection. The measurements are being used to help understand transport and mixing processes, and to form a climatology of aerosol export from North America during the summer months.

  15. How Well Do State-of-the-Art Techniques Measuring the Vertical Profile of Tropospheric Aerosol Extinction Compare?

    SciTech Connect

    Schmid, Beat; Ferrare, Richard; Flynn, Connor M.; Elleman, Robert; Covert, David; Strawa, A.; Welton, E J.; Turner, David D.; Jonsson, Haf; Redemann, Jens; Eilers, J.; Ricci, K.; Hallar, A. G.; Clayton, M. B.; Michalsky, Joseph J.; Smirnov, A.; Holben, B. N.; Barnard, James C.

    2006-02-01

    The recent U.S. Department of Energy Atmospheric Radiation Measurements (ARM) Aerosol Intensive Observation Period (AIOP, May 2003) yielded one of the best measurement sets obtained to-date to assess our ability to measure the vertical profile of ambient aerosol extinction. During one month, a heavily instrumented aircraft with well characterized aerosol sampling ability carrying well proven and new aerosol instrumentation, devoted most of the 60 available flight hours to flying vertical profiles over the heavily instrumented ARM Southern Great Plains (SGP) Climate Research Facility (CRF). This allowed us to compare vertical extinction profiles obtained from 6 different instruments: airborne Sun photometer, airborne nephelometer/absorption photometer, airborne cavity ring-down system, ground-based Raman lidar and two ground-based elastic backscatter lidars. We find the in situ measurements to be biased low (2 - 4 Mm 1 equivalent to 12-17% in the visible, or 45% in the near-infrared) when compared to airborne sunphotometer extinction. On the other hand, we find that with respect to AATS-14, the lidar ?ep(?) are biased high. Bias differences are 0.004 Km-1 (13%) and 0.007 Km-1 (24%) for the two elastic back-scatter lidars (MPLARM and MPLNET, ? = 523 nm) and 0.029 Km-1 (54%) for the Raman lidar (? = 355 nm). An unnoticed loss of sensitivity of the Raman lidar had occurred leading up to AIOP and we expect better agreement from the recently restored system. Looking at the collective results from six field campaigns conducted since 1996, airborne in situ measurements of extinction tend to be biased slightly low (17% at visible wavelengths) when compared to airborne sunphotometer extinction. On the other hand, extinction derived from lidars tend to have no or positive biases. We conclude that the error associated with measuring the tropospheric vertical profile of the ambient aerosol extinction with current state-of-the art instrumentation is 15-20% at visible wavelengths

  16. How Well do State-of-the-Art Techniques Measuring the Vertical Profile of Tropospheric Aerosol Extinction Compare?

    NASA Technical Reports Server (NTRS)

    Schmid, B.; Ferrare, R.; Flynn, C.; Elleman, R.; Covert, D.; Strawa, A.; Welton, E.; Turner, D.; Jonsson, H.; Redemann, J.; Eilers, J.; Ricci, K.; Hallar, A. G.; Clayton, M.; Michalsky, J.; Smirnov, A.; Holben, B.; Barnard, J.

    2006-01-01

    The recent Department of Energy Atmospheric Radiation Measurement (ARM) Aerosol Intensive Operations Period (AIOP, May 2003) yielded one of the best measurement sets obtained to date to assess our ability to measure the vertical profile of ambient aerosol extinction sigma(ep)(lambda) in the lower troposphere. During one month, a heavily instrumented aircraft with well-characterized aerosol sampling ability carrying well-proven and new aerosol instrumentation devoted most of the 60 available flight hours to flying vertical profiles over the heavily instrumented ARM Southern Great Plains (SGP) Climate Research Facility (CRF). This allowed us to compare vertical extinction profiles obtained from six different instruments: airborne Sun photometer (AATS-14), airborne nephelometer/absorption photometer, airborne cavity ring-down system, groundbased Raman lidar, and two ground-based elastic backscatter lidars. We find the in situ measured sigma(ep)(lambda) to be lower than the AATS-14 derived values. Bias differences are 0.002-0.004 Km!1 equivalent to 13-17% in the visible, or 45% in the near-infrared. On the other hand, we find that with respect to AATS-14, the lidar sigma(ep)(lambda) are higher: Bias differences are 0.004 Km(-1) (13%) and 0.007 Km(-1) (24%) for the two elastic backscatter lidars (MPLNET and MPLARM, lambda = 523 nm) and 0.029 Km(-1) (54%) for the Raman lidar (lambda = 355 nm). An unnoticed loss of sensitivity of the Raman lidar had occurred leading up to AIOP, and we expect better agreement from the recently restored system. Looking at the collective results from six field campaigns conducted since 1996, airborne in situ measurements of sigma(ep)(lambda) tend to be biased slightly low (17% at visible wavelengths) when compared to airborne Sun photometer sigma(ep)(lambda). On the other hand, sigma(ep)(lambda) values derived from lidars tend to have no or positive biases. From the bias differences we conclude that the typical systematic error associated

  17. Estimating suspended solids concentrations from backscatter intensity measured by acoustic Doppler current profiler in San Francisco Bay, California

    USGS Publications Warehouse

    Gartner, J.W.

    2004-01-01

    The estimation of mass concentration of suspended solids is one of the properties needed to understand the characteristics of sediment transport in bays and estuaries. However, useful measurements or estimates of this property are often problematic when employing the usual methods of determination from collected water samples or optical sensors. Analysis of water samples tends to undersample the highly variable character of suspended solids, and optical sensors often become useless from biological fouling in highly productive regions. Acoustic sensors, such as acoustic Doppler current profilers that are now routinely used to measure water velocity, have been shown to hold promise as a means of quantitatively estimating suspended solids from acoustic backscatter intensity, a parameter used in velocity measurement. To further evaluate application of this technique using commercially available instruments, profiles of suspended solids concentrations are estimated from acoustic backscatter intensity recorded by 1200- and 2400-kHz broadband acoustic Doppler current profilers located at two sites in San Francisco Bay, California. ADCP backscatter intensity is calibrated using optical backscatterance data from an instrument located at a depth close to the ADCP transducers. In addition to losses from spherical spreading and water absorption, calculations of acoustic transmission losses account for attenuation from suspended sediment and correction for nonspherical spreading in the near field of the acoustic transducer. Acoustic estimates of suspended solids consisting of cohesive and noncohesive sediments are found to agree within about 8-10% (of the total range of concentration) to those values estimated by a second optical backscatterance sensor located at a depth further from the ADCP transducers. The success of this approach using commercially available Doppler profilers provides promise that this technique might be appropriate and useful under certain conditions in

  18. Vertical Profile of Aerosol Properties at Pico Mountain, Azores

    NASA Astrophysics Data System (ADS)

    Wright, K.; Mazzoleni, C.; Mazzoleni, L. R.; Dzepina, K.; Hueber, J.; China, S.; Sharma, N.

    2013-12-01

    Pico Mountain (2325m asl) is a dormant volcano in the archipelago of the Azores1500 km west of Lisbon, Portugal in the North Atlantic. It differs from typical mountain ranges such as the Alps or the Rockies, which are large and present a complex orography. Pico Mountain has a simple cone-like structure with only one main peak and is thousands of kilometers away from any other significant mountain range. In summer months, it is typical for air masses to move around the mountain rather than traveling up its face. This implies that often the peak of the mountain lies above the marine boundary layer in the free troposphere, while the lower part of the mountain is affected by marine clouds and marine air-masses. An atmospheric monitoring station, the Pico Mountain Observatory was established in 2001 in the summit caldera of the volcano at 2225m above sea level. The observatory is far from large populations or pollution sources, which makes the station ideal to study atmospheric gases and aerosols transported over long-ranges in the free troposphere. The station is reachable only by foot following a steep and strenuous hiking trail. In the summer of 2013 we began to collect vertical profiles of aerosol by carrying an instrumented backpack up to the summit of the mountain, with the goal of studying the vertical structure of atmospheric aerosols from the marine boundary layer to the free troposphere. The backpack was carried from the base of trail at 1200m asl. The backpack was equipped with the following instruments: 1. Nephelometer to measure light scattering from aerosol 2. 2-size optical particle counter (300-500 nm) 3. Portable micro-aethalometer to measure absorbing aerosols 4. SEM/TEM sampler to collect particles for off-line electron microscopy analysis 5. Battery powered data logger to measure relative humidity, temperature and pressure 6. GPS tracking device We provide a preliminary analysis of data collected in 2013 to gain insight on the vertical distribution

  19. Deriving Vertical Profiles of Aerosol Sizes from TES

    NASA Astrophysics Data System (ADS)

    Wolff, M. J.; Clancy, R. T.; Smith, M. D.; McConnochie, T. H.; Flittner, D. E.; Fouchet, T.

    2011-12-01

    Vertical variations in aerosol particle sizes can have a dramatic effect in their net impact on the state and evolution of the Martian atmosphere. Recent analyses of data from the Spectroscopy for the Investigation of the Characteristics of the Atmosphere of Mars (SPICAM) and the Thermal Emission Spectrometer (TES) instruments offer some long overdue progress in constraining this aspect of aerosols. However, significantly more work remains to be done along these lines in order to better constrain and inform modern dynamical simulations of the Martian atmosphere. Thus, the primary goal of our work is to perform retrievals of particle size as a function of altitude for both dust and water ice aerosols. The choice of the TES dataset, with pole-to-pole coverage over a period of nearly three martian years, provides the crucial systematic temporal and spatial sampling. Additional leverage on the particle size will be obtained by using both solarband bolometry and infrared (IR) spectroscopy. Our presentation will include: 1) A summary of our limb radiative transfer comparison/validation exercises which include Monte Carlo, Gauss-Seidel, and discrete-ordinate algorithms (including the plane-parallel source function approximation). 2) The initial results of the application of our particle size retrieval scheme to the TES observations of the 2001 planet encircling dust event. 3) A few test applications to the Mars Climate Sounder (MCS) radiance profiles (enabled by the recent solarband radiometric calibration by Bandfield and collaborators). 4) Our plans for additional retrievals (aphelion cloud season, lower optical depth locations and seasons, etc.) and the distribution of the derived profiles.

  20. The Aerosol Limb Imager: acousto-optic imaging of limb scattered sunlight for stratospheric aerosol profiling

    NASA Astrophysics Data System (ADS)

    Elash, B. J.; Bourassa, A. E.; Loewen, P. R.; Lloyd, N. D.; Degenstein, D. A.

    2015-12-01

    The Aerosol Limb Imager (ALI) is an optical remote sensing instrument designed to image scattered sunlight from the atmospheric limb. These measurements are used to retrieve spatially resolved information of the stratospheric aerosol distribution, including spectral extinction coefficient and particle size. Here we present the design, development and test results of an ALI prototype instrument. The long term goal of this work is the eventual realization of ALI on a satellite platform in low earth orbit, where it can provide high spatial resolution observations, both in the vertical and cross-track. The instrument design uses a large aperture Acousto-Optic Tunable Filter (AOTF) to image the sunlit stratospheric limb in a selectable narrow wavelength band ranging from the visible to the near infrared. The ALI prototype was tested on a stratospheric balloon flight from the Canadian Space Agency (CSA) launch facility in Timmins, Canada, in September 2014. Preliminary analysis of the hyperspectral images indicate that the radiance measurements are of high quality, and we have used these to retrieve vertical profiles of stratospheric aerosol extinction coefficient from 650-1000 nm, along with one moment of the particle size distribution. Those preliminary results are promising and development of a satellite prototype of ALI within the Canadian Space Agency is ongoing.

  1. Implementation of Raman lidar for profiling of atmospheric water vapor and aerosols at the Southern Great Plains Cloud and Radiation Testbed Site

    SciTech Connect

    Goldsmith, J.E.M.; Bisson, S.E.; Blair, F.H.; Whiteman, D.N.; Melfi, S.H.

    1995-04-01

    There are clearly identified scientific requirements for continuous profiling of atmospheric water vapor at the Southern Great Plains (SGP) Cloud and Radiation Testbed (CART) site. Research conducted at several laboratories, including our own collaboration in a previous Instrument Development Project for the Atmospheric Radiation Measurement (ARM) Program, has demonstrated the suitability of Raman lidar for providing measurements that are an excellent match to those requirements. We are currently building a rugged Raman lidar system that will reside permanently at the CART site and that is computer-automated to reduce the requirements for operator interaction. In addition to the design goal of profiling water vapor through most of the troposphere during nighttime and through the boundary layer during daytime, the lidar is intended to provide quantitative characterizations of aerosols and clouds, including depolarization measurements for particle phase studies. Raman lidar systems detect selected species by monitoring the wavelength-shifted molecular return produced by Raman scattering from the chosen molecule or molecules. For water-vapor measurements, the nitrogen Raman signal is observed simultaneously with the water-vapor Raman signal; proper ratioing of the signals yields the water-vapor mixing ratio. Similarly, when the backscatter signal at the laser wavelength (which contains contributions from both Rayleigh and aerosol scattering) is also recorded simultaneously, the ratio of the backscatter signal to the nitrogen Raman signal yields a quantitative measurement of the aerosol scattering ratio. A variety of aerosol and cloud parameters can be derived from this measurement. In aerosol-free regions of the atmosphere, temperature profiles can be derived from the density measurements obtained from the nitrogen Raman signal.

  2. Vertical profiling of marine aerosol, dust and their mixtures utilizing the synergy of sunphotometer and lidar measurements

    NASA Astrophysics Data System (ADS)

    Tsekeri, Alexandra; Amiridis, Vassilis; Lopatin, Anton; Marinou, Eleni; Engelman, Ronny; Baars, Holger; Wandinger, Ulla; Ansmann, Albert; Solomos, Stavros; Dubovik, Oleg; Schüttemeyer, Dirk

    2015-04-01

    Current and future lidar products from space missions (CALIPSO, ADM-Aeolus, EarthCARE) aim to improve our understanding of atmospheric dynamics and aerosol/cloud interactions on global scale. However, the lidar instruments onboard these three missions (CALIOP, ALADIN, ATLID) are different systems, operating at different wavelengths and providing different sets of measured parameters. In order to spectrally homogenize the datasets, aerosol/cloud-type-dependent spectral conversion factors are needed to be applied to all lidar-related properties (extinction, backscatter and depolarization), based on the aerosol/cloud classification of the space-borne observations. The well-established European Aerosol Research Lidar Network (EARLINET) offers the unique opportunity to support such an effort. However, EARLINET database suffers from lack of information for specific aerosol types such as marine and mixed dust/marine cases. Unfortunately, these types are not observed in EARLINET's core stations, since the stations are mostly located at continental sites and are influenced by urban pollution. Moreover, the lidar systems near the coastlines suffer from the inability to measure at the first few hundred meters (500-1000 m) due to their technical design, which results in an incomplete laser/telescope overlap region. Towards the study of marine and marine-dust aerosol mixtures we organized the experimental campaign of "Characterization of Aerosol mixtures of Dust And Marine origin" (CHARADMexp), on June 20 to July 10, at Finokalia, Grete, Greece. Our aim was to derive optical, microphysical and chemical properties of the marine component and its mixtures with dust, employing sophisticated instrumentation installed on the site of Finokalia ACTRIS station, where only marine and dust particles are present 95% of the time. Specifically, aerosol characterization was established by the "Generalized Aerosol Retrieval from Radiometer and Lidar Combined data" (GARRLiC), a technique that

  3. Use of In Situ Cloud Condensation Nuclei, Extinction, and Aerosol Size Distribution Measurements to Test a Method for Retrieving Cloud Condensation Nuclei Profiles From Surface Measurements

    NASA Technical Reports Server (NTRS)

    Ghan, Stephen J.; Rissman, Tracey A.; Ellman, Robert; Ferrare, Richard A.; Turner, David; Flynn, Connor; Wang, Jian; Ogren, John; Hudson, James; Jonsson, Haflidi H.; VanReken, Timothy; Flagan, Richard C.; Seinfeld, John H.

    2006-01-01

    If the aerosol composition and size distribution below cloud are uniform, the vertical profile of cloud condensation nuclei (CCN) concentration can be retrieved entirely from surface measurements of CCN concentration and particle humidification function and surface-based retrievals of relative humidity and aerosol extinction or backscatter. This provides the potential for long-term measurements of CCN concentrations near cloud base. We have used a combination of aircraft, surface in situ, and surface remote sensing measurements to test various aspects of the retrieval scheme. Our analysis leads us to the following conclusions. The retrieval works better for supersaturations of 0.1% than for 1% because CCN concentrations at 0.1% are controlled by the same particles that control extinction and backscatter. If in situ measurements of extinction are used, the retrieval explains a majority of the CCN variance at high supersaturation for at least two and perhaps five of the eight flights examined. The retrieval of the vertical profile of the humidification factor is not the major limitation of the CCN retrieval scheme. Vertical structure in the aerosol size distribution and composition is the dominant source of error in the CCN retrieval, but this vertical structure is difficult to measure from remote sensing at visible wavelengths.

  4. Vertical microphysical profiles of convective clouds as a tool for obtaining aerosol cloud-mediated climate forcings

    SciTech Connect

    Rosenfeld, Daniel

    2015-12-23

    Quantifying the aerosol/cloud-mediated radiative effect at a global scale requires simultaneous satellite retrievals of cloud condensation nuclei (CCN) concentrations and cloud base updraft velocities (Wb). Hitherto, the inability to do so has been a major cause of high uncertainty regarding anthropogenic aerosol/cloud-mediated radiative forcing. This can be addressed by the emerging capability of estimating CCN and Wb of boundary layer convective clouds from an operational polar orbiting weather satellite. Our methodology uses such clouds as an effective analog for CCN chambers. The cloud base supersaturation (S) is determined by Wb and the satellite-retrieved cloud base drop concentrations (Ndb), which is the same as CCN(S). Developing and validating this methodology was possible thanks to the ASR/ARM measurements of CCN and vertical updraft profiles. Validation against ground-based CCN instruments at the ARM sites in Oklahoma, Manaus, and onboard a ship in the northeast Pacific showed a retrieval accuracy of ±25% to ±30% for individual satellite overpasses. The methodology is presently limited to boundary layer not raining convective clouds of at least 1 km depth that are not obscured by upper layer clouds, including semitransparent cirrus. The limitation for small solar backscattering angles of <25º restricts the satellite coverage to ~25% of the world area in a single day. This methodology will likely allow overcoming the challenge of quantifying the aerosol indirect effect and facilitate a substantial reduction of the uncertainty in anthropogenic climate forcing.

  5. Novel Co:MgF2 lidar for aerosol profiler

    NASA Technical Reports Server (NTRS)

    Acharekar, M. A.

    1993-01-01

    Lidars are of great interest because of their unique capabilities in remote sensing applications in sounding of the atmosphere, meteorology, and climatology. In this small business innovative research (SBIR) phase II program, laser sources including Co:MgF2, CTH:YAG, CTH:YSGG, CT:YAG, and Er:Glass were evaluated. Modulator of fused silica and TeO2 materials with Brewster's angle end faces were used with these lasers as acousto-optical (AO) Q-switches. A higher hold-off energy and hence a higher Q-switched energy was obtained by using a high power RF driver. The report provides performance characteristics of these lasers. The tunable (1.75-2.50 microns) Co:MgF2 laser damaged the TeO2 Q-switch cell. However, the CTH:YAG laser operating at 2.09 microns provided output energy of over 300 mJ/p in 50 ns pulse width using the fused silica Q-switch. This Q-switched CTH:YAG laser was used in a breadboard vertical aerosol profiler. A 40 cm diameter telescope, InSb and InGaAs detectors were used in the receiver. The data obtained using this lidar is provided in the report. The data shows that the eye safe lidar using CTH:YAG laser for the vertical aerosol density and range measurements is the viable approach.

  6. Retrieving the aerosol lidar ratio profile by combining ground- and space-based elastic lidars.

    PubMed

    Feiyue, Mao; Wei, Gong; Yingying, Ma

    2012-02-15

    The aerosol lidar ratio is a key parameter for the retrieval of aerosol optical properties from elastic lidar, which changes largely for aerosols with different chemical and physical properties. We proposed a method for retrieving the aerosol lidar ratio profile by combining simultaneous ground- and space-based elastic lidars. The method was tested by a simulated case and a real case at 532 nm wavelength. The results demonstrated that our method is robust and can obtain accurate lidar ratio and extinction coefficient profiles. Our method can be useful for determining the local and global lidar ratio and validating space-based lidar datasets.

  7. Infrared lidar observations of stratospheric aerosols.

    PubMed

    Forrister, H N; Roberts, D W; Mercer, A J; Gimmestad, G G

    2014-06-01

    We observed the stratospheric aerosol layer at 34° north latitude with a photon-counting 1574 nm lidar on three occasions in 2011. During all of the observations, we also operated a nearby 523.5 nm micropulse lidar and acquired National Weather Service upper air data. We analyzed the lidar data to find scattering ratio profiles and the integrated aerosol backscatter at both wavelengths and then calculated the color ratio and wavelength exponent for lidar backscattering from the stratospheric aerosols. The visible-light integrated backscatter values of the layer were in the range 2.8-3.5×10⁻⁴ sr⁻¹ and the infrared integrated backscatter values ranged from 2.4 to 3.7×10⁻⁵  sr⁻¹. The wavelength exponent was determined to be 1.9±0.2.

  8. Comparison of aerosol extinction profiles from lidar and SAGE II data at a tropical station

    NASA Technical Reports Server (NTRS)

    Parameswaran, K.; Rose, K. O.; Murthy, B. V. K.; Osborn, M. T.; Mcmaster, L. R.

    1991-01-01

    Aerosol extinction profiles obtained from lidar data at Trivandrum (8.6 deg N, 77 deg E) are compared with corresponding Stratospheric Aerosol and Gas Experiment II extinction profiles. The agreement between the two is found to be satisfactory. The extinction profiles obtained by both the experiments showed a prominent peak at 23-24 km altitude in the stratosphere. The study revealed large variability in upper tropospheric extinction with location (latitude).

  9. Light scattering characteristics of various aerosol types derived from multiple wavelength lidar observations

    NASA Technical Reports Server (NTRS)

    Sasano, Yasuhiro; Browell, Edward V.

    1989-01-01

    The present study demonstrates the potential of a multiple-wavelength lidar for discriminating between several aerosol types on the basis of the wavelength dependence of the aerosol backscatter coefficient. The two-component lidar equation was solved under the assumption of similarity in the derived profiles of backscatter coefficients for each wavelength. It is shown that a three-wavelength lidar system operating at 300, 600, and 1064nm can provide unique information for discriminating between various aerosol types (continental, maritime, Saharan-dust, stratospheric aerosols in a tropopause fold event, and tropical forest aerosols). Mie calculations were made using in situ aerosol data and aerosol models to compare with the lidar results. The disagreement between the theoretical and empirical results in some cases was substantial. These differences may be partly due to uncertainties in the lidar data analysis and aerosol characteristics and also due to the conventional assumption of aerosol sphericity for the aerosol Mie calculations.

  10. Vertical profiles of cloud condensation nuclei, aerosol hygroscopicity, water uptake, and scattering across the United States

    NASA Astrophysics Data System (ADS)

    Lin, J. J.; Bougiatioti, A.; Nenes, A.; Anderson, B. E.; Beyersdorf, A. J.; Brock, C. A.; Gordon, T. D.; Lack, D.; Law, D. C.; Liao, J.; Middlebrook, A. M.; Richardson, M.; Thornhill, K. L., II; Winstead, E.; Wagner, N. L.; Welti, A.; Ziemba, L. D.

    2014-12-01

    The evolutions of vertical distributions of aerosol chemical, microphysical, hygroscopic, and optical properties present fundamental challenges to the understanding of ground-level air quality and radiative transfer, and few datasets exist to date for evaluation of atmospheric models. Data collected from recent NASA and NOAA field campaigns in the California Central Valley (DISCOVER-AQ), southeast United States (SENEX, SEAC4RS) and Texas (DISCOVER-AQ) allow for a unique opportunity to constrain vertical profiles of climate-relevant aerosol properties. This work presents in-situ aircraft measurements of cloud condensation nuclei (CCN) concentration and derivations of aerosol hygroscopicity, water uptake, and light scattering. Aerosol hygroscopicity is derived from CCN and aerosol measurements. Inorganic water uptake is calculated from aerosol composition using ISORROPIA, a chemical thermodynamic model, while organic water uptake is calculated from organic hygroscopicity. Aerosol scattering closure is performed between scattering from water uptake calculations and in-situ scattering measurements.

  11. Potential of polarization lidar to provide profiles of CCN- and INP-relevant aerosol parameters

    NASA Astrophysics Data System (ADS)

    Mamouri, R. E.; Ansmann, A.

    2015-12-01

    We investigate the potential of polarization lidar to provide vertical profiles of aerosol parameters from which cloud condensation nucleus (CCN) and ice nucleating particle (INP) number concentrations can be estimated. We show that height profiles of number concentrations of aerosol particles with radius > 50 nm (APC50, reservoir of favorable CCN) and with radius > 250 nm (APC250, reservoir of favorable INP), as well as profiles of the aerosol particle surface area concentration (ASC, used in INP parameterization) can be retrieved from lidar-derived aerosol extinction coefficients (AEC) with relative uncertainties of a factor of around 2 (APC50), and of about 25-50 % (APC250, ASC). Of key importance is the potential of polarization lidar to identify mineral dust particles and to distinguish and separate the aerosol properties of basic aerosol types such as mineral dust and continental pollution (haze, smoke). We investigate the relationship between AEC and APC50, APC250, and ASC for the main lidar wavelengths of 355, 532 and 1064 nm and main aerosol types (dust, pollution, marine). Our study is based on multiyear Aerosol Robotic Network (AERONET) photometer observations of aerosol optical thickness and column-integrated particle size distribution at Leipzig, Germany, and Limassol, Cyprus, which cover all realistic aerosol mixtures of continental pollution, mineral dust, and marine aerosol. We further include AERONET data from field campaigns in Morocco, Cabo Verde, and Barbados, which provide pure dust and pure marine aerosol scenarios. By means of a simple relationship between APC50 and the CCN-reservoir particles (APCCCN) and published INP parameterization schemes (with APC250 and ASC as input) we finally compute APCCCN and INP concentration profiles. We apply the full methodology to a lidar observation of a heavy dust outbreak crossing Cyprus with dust up to 8 km height and to a case during which anthropogenic pollution dominated.

  12. Vertical Profiles of Aerosol Volume from High Spectral Resolution Infrared Transmission Measurements: Results

    NASA Technical Reports Server (NTRS)

    Eldering, Annmarie; Kahn, Brian H.; Mills, Franklin P.; Irion, Fredrick W.; Steele, Helen M.; Gunson, Michael R.

    2004-01-01

    The high-resolution infrared absorption spectra of the Atmospheric Trace Molecule Spectroscopy (ATMOS) experiment are utilized to derive vertical profiles of sulfate aerosol volume density and extinction coefficient. Following the eruption of Mt. Pinatubo in June 1991, the ATMOS spectra obtained on three Space Shuttle missions (1992, 1993, and 1994) provide a unique opportunity to study the global stratospheric sulfate aerosol layer shortly after a major volcanic eruption and periodically during the decay phase. Synthetic sulfate aerosol spectra are fit to the observed spectra, and a global fitting inversion routine is used to derive vertical profiles of sulfate aerosol volume density. Vertical profiles of sulfate aerosol volume density for the three missions over portions of the globe are presented, with the peak in aerosol volume density occurring from as low as 10 km (polar latitudes) to as high as 20 km (subtropical latitudes). Derived aerosol volume density is as high as 2-3.5 (mu)m(exp 3) per cubic centimeter +/-10% in 1992, decreasing to 0.2-0.5 (mu)m(exp 3) per cubic centimeter +/-20% in 1994, in agreement with other experiments. Vertical extinction profiles derived from ATMOS are compared with profiles from Improved Stratospheric And Mesospheric Sounder (ISAMS) and Cryogenic Limb Array Etalon Spectrometer (CLAES) that coincide in space and time and show good general agreement. The uncertainty of the ATMOS vertical profiles is similar to CLAES and consistently smaller than ISAMS at similar altitudes.

  13. The effect of aerosol vertical profiles on satellite-estimated surface particle sulfate concentrations

    SciTech Connect

    Liu, Yang; Wang, Zifeng; Wang, Jun; Ferrare, Richard A.; Newsom, Rob K.; Welton, Ellsworth J.

    2011-02-15

    The aerosol vertical distribution is an important factor in determining the relationship between satellite retrieved aerosol optical depth (AOD) and ground-level fine particle pollution concentrations. We evaluate how aerosol profiles measured by ground-based lidar and simulated by models can help improve the association between AOD retrieved by the Multi-angle Imaging Spectroradiometer (MISR) and fine particle sulfate (SO4) concentrations using matched data at two lidar sites. At the Goddard Space Flight Center (GSFC) site, both lidar and model aerosol profiles marginally improve the association between SO4 concentrations and MISR fractional AODs, as the correlation coefficient between cross-validation (CV) and observed SO4 concentrations changes from 0.87 for the no-scaling model to 0.88 for models scaled with aerosol vertical profiles. At the GSFC site, a large amount of urban aerosols resides in the well-mixed boundary layer so the column fractional AODs are already excellent indicators of ground-level particle pollution. In contrast, at the Atmospheric Radiation Measurement Program (ARM) site with relatively low aerosol loadings, scaling substantially improves model performance. The correlation coefficient between CV and observed SO4 concentrations is increased from 0.58 for the no-scaling model to 0.76 in the GEOS-Chem scaling model, and the model bias is reduced from 17% to 9%. In summary, despite the inaccuracy due to the coarse horizontal resolution and the challenges of simulating turbulent mixing in the boundary layer, GEOS-Chem simulated aerosol profiles can still improve methods for estimating surface aerosol (SO4) mass from satellite-based AODs, particularly in rural areas where aerosols in the free troposphere and any long-range transport of aerosols can significantly contribute to the column AOD.

  14. A comparison of SAGE 1, SBUV, and Umkehr ozone profiles including a search for Umkehr aerosol effects

    NASA Technical Reports Server (NTRS)

    Newchurch, M. J.; Grams, G. W.; Cunnold, D. M.; Deluisi, J. J.

    1987-01-01

    Using a spatially weighted average for the stratospheric aerosol and gas experiment 1 (SAGE 1) events derived from an autocorrelation analysis, 337 colocated SAGE 1 and Umkehr ozone profiles are found. The total column ozone in layers two through nine measured by SAGE 1 is found to be 4.6 + or - 1.3 percent higher at the 95 percent confidence level than the approximate total column ozone measured by Umkehr. Average layer ozone differences indicate that most of this discrepancy resides in the lower layers. Intercomparison of SAGE 1, Nimbus 7 solar backscattered ultraviolet (SBUV), and Umkehr ozone at stations north of 30 deg indicates that, in layer six, Umkehr values are consistently higher than both SAGE 1 and SBUV by about 10 percent. In layer eight, SBUV ozone is higher than both SAGE 1 and SBUV by about 10 percent. In the upper stratosphere, the SAGE 1-Umkehr ozone differences are small for low stratospheric aerosol optical depth cases, but vary from -3 percent in layer six to -8 percent in layer nine for high optical depth cases.

  15. Iterative method for the inversion of multiwavelength lidar signals to determine aerosol size distribution.

    PubMed

    Rajeev, K; Parameswaran, K

    1998-07-20

    Two iterative methods of inverting lidar backscatter signals to determine altitude profiles of aerosol extinction and altitude-resolved aerosol size distribution (ASD) are presented. The first method is for inverting two-wavelength lidar signals in which the shape of the ASD is assumed to be of power-law type, and the second method is for inverting multiwavelength lidar signals without assuming any a priori analytical form of ASD. An arbitrary value of the aerosol extinction-to-backscatter ratio (S(1)) is assumed initially to invert the lidar signals, and the ASD determined by use of the spectral dependence of the retrieved aerosol extinction coefficients is used to improve the value of S(1) iteratively. The methods are tested for different forms of altitude-dependent ASD's by use of simulated lidar-backscatter-signal profiles. The effect of random noise on the lidar backscatter signals is also studied.

  16. Hemispheric aerosol vertical profiles: anthropogenic impacts on optical depth and cloud nuclei.

    PubMed

    Clarke, Antony; Kapustin, Vladimir

    2010-09-17

    Understanding the effect of anthropogenic combustion upon aerosol optical depth (AOD), clouds, and their radiative forcing requires regionally representative aerosol profiles. In this work, we examine more than 1000 vertical profiles from 11 major airborne campaigns in the Pacific hemisphere and confirm that regional enhancements in aerosol light scattering, mass, and number are associated with carbon monoxide from combustion and can exceed values in unperturbed regions by more than one order of magnitude. Related regional increases in a proxy for cloud condensation nuclei (CCN) and AOD imply that direct and indirect aerosol radiative effects are coupled issues linked globally to aged combustion. These profiles constrain the influence of combustion on regional AOD and CCN suitable for challenging climate model performance and informing satellite retrievals.

  17. Radiosonde aerosol counter for vertical profiling of atmospheric dust layers

    NASA Astrophysics Data System (ADS)

    Ulanowski, Z.; Hirst, E.; Kaye, P. H.; Harrison, R. G.; Nicoll, K. A.; Rogers, G.

    2010-05-01

    A low-cost, miniature aerosol particle counter has been developed, intended for use with balloon-borne meteorological radiosondes. It is particularly suitable for airborne mineral dust measurements. Ambient air is drawn into the counter using a diaphragm pump at a rate of 0.5 litre per minute. The counter detects particles in the airstream using a diode laser and a photodiode. Output from the photodiode is digitised into 5 size bins, with minimum particle diameters equivalent to 0.6, 1.4, 2.6, 5.4 and 10.6 micrometers. The counter is interfaced to a Vaisala RS92 radiosonde, which transmits data from the counter together with meteorological parameters and GPS-derived position to a ground based receiver at 1 Hz rate. Statistically significant particle size distributions can be obtained once a second for number concentrations down to about 100,000 particle per litre (within the measured size range), or correspondingly less at lower temporal resolutions. At the same time, the counter is capable of measuring dust number concentrations exceeding a million per litre without incurring significant errors. Soundings during the DREAME campaign in Kuwait (Ulanowski et al. EGU 2010, AS4.7) and on Cape Verde Islands (Nicoll et al. EGU 2010, AS4.7) provided dust concentration profiles with a typical vertical resolution of 4 m. Comparisons with integrated dust column size distribution measurements from AERONET sun photometers showed good agreement in two out of three cases where near-simultaneous retrievals were available. Optical thickness calculations based on the size distributions measured in Kuwait, with the assumption that the dust particles were prolate spheroids, agreed with the AERONET optical thickness at 675 nm to within 15%.

  18. Tropospheric aerosol profile information from high-resolution oxygen A-band measurements from space

    NASA Astrophysics Data System (ADS)

    Geddes, A.; Bösch, H.

    2015-02-01

    Aerosols are an important factor in the Earth climatic system and they play a key role in air quality and public health. Observations of the oxygen A-band at 760 nm can provide information on the vertical distribution of aerosols from passive satellite sensors that can be of great interest for operational monitoring applications with high spatial coverage if the aerosol information is obtained with sufficient precision, accuracy and vertical resolution. To address this issue, retrieval simulations of the aerosol vertical profile retrieval from O2 A-band observations by GOSAT, the upcoming Orbiting Carbon Observatory-2 (OCO-2) and Sentinel 5-P missions, and the proposed CarbonSat mission have been carried out. Precise retrievals of aerosol optical depth (AOD) within the boundary layer were found to favour low-resolution, high signal-to-noise instruments such as Sentinel-5 P, whereas higher-resolution instruments such as OCO-2 showed greater performance at higher altitudes and in information content above the boundary layer. Retrieval of the AOD in the 0-2 km range with precision appears difficult from all studied instruments and the retrieval errors typically exceed a value of 0.05 for AODs up to 0.3. Constraining the surface albedo is a promising and effective way of improving the retrieval of aerosol, but the accuracy of the required prior knowledge is very high. Due to the limited information content of the aerosol profile retrieval, the use of a parameterised aerosol distribution is assessed, and we show that the AOD and height of an aerosol layer can be retrieved well if the aerosol layer is uplifted to the free troposphere; however, errors are often large for aerosol layers in the boundary layer. Additional errors are introduced by incorrect assumptions on surface pressure and aerosol mixture, which can both bias retrieved AOD and height by up to 45%. In addition, assumptions of the boundary layer temperature are found to yield an additional error of up to 8

  19. Vertical profiles of aerosol volume from high-spectral-resolution infrared transmission measurements. I. Methodology.

    PubMed

    Eldering, A; Irion, F W; Chang, A Y; Gunson, M R; Mills, F P; Steele, H M

    2001-06-20

    The wavelength-dependent aerosol extinction in the 800-1250-cm(-1) region has been derived from ATMOS (atmospheric trace molecule spectroscopy) high-spectral-resolution IR transmission measurements. Using models of aerosol and cloud extinction, we have performed weighted nonlinear least-squares fitting to determine the aerosol-volume columns and vertical profiles of stratospheric sulfate aerosol and cirrus cloud volume. Modeled extinction by use of cold-temperature aerosol optical constants for a 70-80% sulfuric-acid-water solution shows good agreement with the measurements, and the derived aerosol volumes for a 1992 occultation are consistent with data from other experiments after the eruption of Mt. Pinatubo. The retrieved sulfuric acid aerosol-volume profiles are insensitive to the aerosol-size distribution and somewhat sensitive to the set of optical constants used. Data from the nonspherical cirrus extinction model agree well with a 1994 mid-latitude measurement indicating the presence of cirrus clouds at the tropopause.

  20. Potential of polarization lidar to provide profiles of CCN- and INP-relevant aerosol parameters

    NASA Astrophysics Data System (ADS)

    Mamouri, Rodanthi-Elisavet; Ansmann, Albert

    2016-05-01

    We investigate the potential of polarization lidar to provide vertical profiles of aerosol parameters from which cloud condensation nucleus (CCN) and ice nucleating particle (INP) number concentrations can be estimated. We show that height profiles of particle number concentrations n50, dry considering dry aerosol particles with radius > 50 nm (reservoir of CCN in the case of marine and continental non-desert aerosols), n100, dry (particles with dry radius > 100 nm, reservoir of desert dust CCN), and of n250, dry (particles with dry radius > 250 nm, reservoir of favorable INP), as well as profiles of the particle surface area concentration sdry (used in INP parameterizations) can be retrieved from lidar-derived aerosol extinction coefficients σ with relative uncertainties of a factor of 1.5-2 in the case of n50, dry and n100, dry and of about 25-50 % in the case of n250, dry and sdry. Of key importance is the potential of polarization lidar to distinguish and separate the optical properties of desert aerosols from non-desert aerosol such as continental and marine particles. We investigate the relationship between σ, measured at ambient atmospheric conditions, and n50, dry for marine and continental aerosols, n100, dry for desert dust particles, and n250, dry and sdry for three aerosol types (desert, non-desert continental, marine) and for the main lidar wavelengths of 355, 532, and 1064 nm. Our study is based on multiyear Aerosol Robotic Network (AERONET) photometer observations of aerosol optical thickness and column-integrated particle size distribution at Leipzig, Germany, and Limassol, Cyprus, which cover all realistic aerosol mixtures. We further include AERONET data from field campaigns in Morocco, Cabo Verde, and Barbados, which provide pure dust and pure marine aerosol scenarios. By means of a simple CCN parameterization (with n50, dry or n100, dry as input) and available INP parameterization schemes (with n250, dry and sdry as input) we finally compute

  1. Final Technical Report. Cloud and Radiation Testbed (CART) Raman Lidar measurement of atmospheric aerosols for the Atmospheric Radiation Measurement (ARM) Program

    SciTech Connect

    Ferrare, Richard A.

    2002-08-19

    Vertical profiles of aerosol extinction are required for determination of the effects of aerosols on the clear-sky radiative flux. Since recent studies have demonstrated the inability to compute these profiles on surface aerosol measurements alone, vertical profiles of aerosol optical properties must be acquired to compute aerosol radiative effects throughout the entire atmospheric column. Following the recommendation of the ARM Aerosol Working Group, the investigator developed, evaluated, and implemented algorithms for the CART Raman Lidar to provide profiles of aerosol extinction and backscattering. By virtue of its ability to measure vertical profiles of both aerosol extinction and water vapor simultaneously in the same scattering volume, we used the resulting profiles from the CART Raman Lidar to investigate the impact of water vapor and relative humidity on aerosol extinction throughout the column on a continuous and routine basis. The investigator used these the CART Raman Lidar aerosol extinction and backscattering profiles to evaluate the vertical variability of aerosol extinction and the extinction/backscatter ratio over the ARM SGP site.

  2. An overview of the first decade of PollyNET: an emerging network of automated Raman-polarization lidars for continuous aerosol profiling

    NASA Astrophysics Data System (ADS)

    Baars, Holger; Kanitz, Thomas; Engelmann, Ronny; Althausen, Dietrich; Heese, Birgit; Komppula, Mika; Preißler, Jana; Tesche, Matthias; Ansmann, Albert; Wandinger, Ulla; Lim, Jae-Hyun; Ahn, Joon Young; Stachlewska, Iwona S.; Amiridis, Vassilis; Marinou, Eleni; Seifert, Patric; Hofer, Julian; Skupin, Annett; Schneider, Florian; Bohlmann, Stephanie; Foth, Andreas; Bley, Sebastian; Pfüller, Anne; Giannakaki, Eleni; Lihavainen, Heikki; Viisanen, Yrjö; Hooda, Rakesh Kumar; Nepomuceno Pereira, Sérgio; Bortoli, Daniele; Wagner, Frank; Mattis, Ina; Janicka, Lucja; Markowicz, Krzysztof M.; Achtert, Peggy; Artaxo, Paulo; Pauliquevis, Theotonio; Souza, Rodrigo A. F.; Prakesh Sharma, Ved; Gideon van Zyl, Pieter; Beukes, Johan Paul; Sun, Junying; Rohwer, Erich G.; Deng, Ruru; Mamouri, Rodanthi-Elisavet; Zamorano, Felix

    2016-04-01

    A global vertically resolved aerosol data set covering more than 10 years of observations at more than 20 measurement sites distributed from 63° N to 52° S and 72° W to 124° E has been achieved within the Raman and polarization lidar network PollyNET. This network consists of portable, remote-controlled multiwavelength-polarization-Raman lidars (Polly) for automated and continuous 24/7 observations of clouds and aerosols. PollyNET is an independent, voluntary, and scientific network. All Polly lidars feature a standardized instrument design with different capabilities ranging from single wavelength to multiwavelength systems, and now apply unified calibration, quality control, and data analysis. The observations are processed in near-real time without manual intervention, and are presented online at http://polly.tropos.de/. The paper gives an overview of the observations on four continents and two research vessels obtained with eight Polly systems. The specific aerosol types at these locations (mineral dust, smoke, dust-smoke and other dusty mixtures, urban haze, and volcanic ash) are identified by their Ångström exponent, lidar ratio, and depolarization ratio. The vertical aerosol distribution at the PollyNET locations is discussed on the basis of more than 55 000 automatically retrieved 30 min particle backscatter coefficient profiles at 532 nm as this operating wavelength is available for all Polly lidar systems. A seasonal analysis of measurements at selected sites revealed typical and extraordinary aerosol conditions as well as seasonal differences. These studies show the potential of PollyNET to support the establishment of a global aerosol climatology that covers the entire troposphere.

  3. Vertical Profiles of Aerosol Optical Properties Over Central Illinois and Comparison with Surface and Satellite Measurements

    NASA Technical Reports Server (NTRS)

    Sheridan P. J.; Andrews, E.; Ogren, J A.; Tackett, J. L.; Winker, D. M.

    2012-01-01

    Between June 2006 and September 2009, an instrumented light aircraft measured over 400 vertical profiles of aerosol and trace gas properties over eastern and central Illinois. The primary objectives of this program were to (1) measure the in situ aerosol properties and determine their vertical and temporal variability and (2) relate these aircraft measurements to concurrent surface and satellite measurements. Underflights of the CALIPSO satellite show reasonable agreement in a majority of retrieved profiles between aircraft-measured extinction at 532 nm (adjusted to ambient relative humidity) and CALIPSO-retrieved extinction, and suggest that routine aircraft profiling programs can be used to better understand and validate satellite retrieval algorithms. CALIPSO tended to overestimate the aerosol extinction at this location in some boundary layer flight segments when scattered or broken clouds were present, which could be related to problems with CALIPSO cloud screening methods. The in situ aircraft-collected aerosol data suggest extinction thresholds for the likelihood of aerosol layers being detected by the CALIOP lidar. These statistical data offer guidance as to the likelihood of CALIPSO's ability to retrieve aerosol extinction at various locations around the globe.

  4. Improved stratospheric aerosol extinction profiles from SCIAMACHY: validation and sample results

    NASA Astrophysics Data System (ADS)

    von Savigny, C.; Ernst, F.; Rozanov, A.; Hommel, R.; Eichmann, K.-U.; Rozanov, V.; Burrows, J. P.; Thomason, L. W.

    2015-12-01

    Stratospheric aerosol extinction profiles have been retrieved from SCIAMACHY/Envisat measurements of limb-scattered solar radiation. The retrieval is an improved version of an algorithm presented earlier. The retrieved aerosol extinction profiles are compared to co-located aerosol profile measurements from the SAGE II solar occultation instrument at a wavelength of 525 nm. Comparisons were carried out with two versions of the SAGE II data set (version 6.2 and the new version 7.0). In a global average sense the SCIAMACHY and the SAGE II version 7.0 extinction profiles agree to within about 10 % for altitudes above 15 km. Larger relative differences (up to 40 %) are observed at specific latitudes and altitudes. We also find differences between the two SAGE II data versions of up to 40 % for specific latitudes and altitudes, consistent with earlier reports. Sample results on the latitudinal and temporal variability of stratospheric aerosol extinction and optical depth during the SCIAMACHY mission period are presented. The results confirm earlier reports that a series of volcanic eruptions is responsible for the increase in stratospheric aerosol optical depth from 2002 to 2012. Above about an altitude of 28 km, volcanic eruptions are found to have negligible impact in the period 2002-2012.

  5. Vertical distribution of aerosol extinction cross section and inference of aerosol imaginary index in the troposphere by lidar technique

    NASA Technical Reports Server (NTRS)

    Spinhirne, J. D.; Reagan, J. A.; Herman, B. M.

    1980-01-01

    The paper reports on vertical profiles of aerosol extinction and backscatter in the troposphere which were obtained from multi zenith angle lidar measurements. It is reported that a direct slant path solution was found to be not possible due to horizontal inhomogeneity of the atmosphere. Attention is given to the use of a regression analysis with respect to zenith angle for a layer integration of the angle dependent lidar equation in order to determine the optical thickness and aerosol extinction-to-backscatter ratio for defined atmospheric layers and the subsequent evaluation of cross-section profiles.

  6. Characterizing the vertical profile of aerosol particle extinction and linear depolarization over Southeast Asia and the Maritime Continent: The 2007-2009 view from CALIOP

    NASA Astrophysics Data System (ADS)

    Campbell, James R.; Reid, Jeffrey S.; Westphal, Douglas L.; Zhang, Jianglong; Tackett, Jason L.; Chew, Boon Ning; Welton, Ellsworth J.; Shimizu, Atsushi; Sugimoto, Nobuo; Aoki, Kazuma; Winker, David M.

    2013-03-01

    Vertical profiles of 0.532 μm aerosol particle extinction coefficient and linear volume depolarization ratio are described for Southeast Asia and the Maritime Continent. Quality-screened and cloud-cleared Version 3.01 Level 2 NASA Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) 5-km Aerosol Profile datasets are analyzed from 2007 to 2009. Numerical simulations from the U.S. Naval Aerosol Analysis and Predictive System (NAAPS), featuring two-dimensional variational assimilation of NASA Moderate Resolution Imaging Spectroradiometer and Multi-angle Imaging SpectroRadiometer quality-assured datasets, combined with regional ground-based lidar measurements, are considered for assessing CALIOP retrieval performance, identifying bias, and evaluating regional representativeness. CALIOP retrievals of aerosol particle extinction coefficient and aerosol optical depth (AOD) are high over land and low over open waters relative to NAAPS (0.412/0.312 over land for all data points inclusive, 0.310/0.235 when the per bin average is used and each is treated as single data points; 0.102/0.151 and 0.086/0.124, respectively, over ocean). Regional means, however, are very similar (0.180/0.193 for all data points and 0.155/0.159 when averaged per normalized bin), as the two factors offset one another. The land/ocean offset is investigated, and discrepancies attributed to interpretation of particle composition and a-priori assignment of the extinction-to-backscatter ratio (“lidar ratio”) necessary for retrieving the extinction coefficient from CALIOP signals. Over land, NAAPS indicates more dust present than CALIOP algorithms are identifying, indicating a likely assignment of a higher lidar ratio representative of more absorptive particles. NAAPS resolves more smoke over water than identified with CALIOP, indicating likely usage of a lidar ratio characteristic of less absorptive particles to be applied that biases low AOD there. Over open waters except within the Bay of

  7. Characterizing the Vertical Profile of Aerosol Particle Extinction and Linear Depolarization over Southeast Asia and the Maritime Continent: The 2007-2009 View from CALIOP

    NASA Technical Reports Server (NTRS)

    Campbell, James R.; Reid, Jeffrey S.; Westphal, Douglas L.; Zhang, Jianglong; Tackett, Jason L.; Chew, Boon Ning; Welton, Ellsworth J.; Shimizu, Atsushi; Sugimoto, Nobuo; Aoki, Kazuma; Winker, David M.

    2012-01-01

    Vertical profiles of 0.532 µm aerosol particle extinction coefficient and linear volume depolarization ratio are described for Southeast Asia and the Maritime Continent. Quality-screened and cloud-cleared Version 3.01 Level 2 NASA Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) 5-km Aerosol Profile datasets are analyzed from 2007 to 2009. Numerical simulations from the U.S. Naval Aerosol Analysis and Predictive System (NAAPS), featuring two-dimensional variational assimilation of NASA Moderate Resolution Imaging Spectroradiometer and Multi-angle Imaging Spectro- Radiometer quality-assured datasets, combined with regional ground-based lidar measurements, are considered for assessing CALIOP retrieval performance, identifying bias, and evaluating regional representativeness. CALIOP retrievals of aerosol particle extinction coefficient and aerosol optical depth (AOD) are high over land and low over open waters relative to NAAPS (0.412/0.312 over land for all data points inclusive, 0.310/0.235 when the per bin average is used and each is treated as single data points; 0.102/0.151 and 0.086/0.124, respectively, over ocean). Regional means, however, are very similar (0.180/0.193 for all data points and 0.155/0.159 when averaged per normalized bin), as the two factors offset one another. The land/ocean offset is investigated, and discrepancies attributed to interpretation of particle composition and a-priori assignment of the extinction-to-backscatter ratio ("lidar ratio") necessary for retrieving the extinction coefficient from CALIOP signals. Over land, NAAPS indicates more dust present than CALIOP algorithms are identifying, indicating a likely assignment of a higher lidar ratio representative of more absorptive particles. NAAPS resolvesmore smoke overwater than identified with CALIOP, indicating likely usage of a lidar ratio characteristic of less absorptive particles to be applied that biases low AOD there. Over open waters except within the Bay of Bengal

  8. [Dual-wavelength Mie lidar observations of tropospheric aerosols].

    PubMed

    Chi, Ru-Li; Wu, De-Cheng; Liu, Bo; Zhou, Jun

    2009-06-01

    A new dual-wavelength Mie lidar (DWL) is introduced. The DWL can be used to monitor the optical properties of tropospheric aerosol at 532 and 1 064 nm wavelength and their spatial and temporal variations, and to research aerosol size distribution with altitude. This lidar adopted four channels to receive the far and near range backscattering signal at 532 and 1 064 nm wavelength respectively. In order to enhance the capability of daytime measurement, the system employed a narrow band interference filter to separate the main backscattering signal of lidar return, including Mie backscattering signal and Rayleigh backscattering signal from the total backscattering signal including non-elastic scattering signal and solar spectrum, by cooperating with an iris to depress the majority of sky background noise. Overall structure and specifications of the lidar, as well as data processing method, were described. The lidar system has been operated in Hefei (117. 16 degrees E, 31.90 degrees N). The profile of extinction coefficient of tropospheric aerosol and its temporal-spatial distribution were obtained. Angstrom exponent and optical depth of aerosol were also discussed. The observational results have shown that this lidar works well both during the day and at night and has the ability to measure the tropospheric aerosols and to manifest the temporal and spatial distributions of the aerosols with high precision.

  9. Profile and Morphology of Fungal Aerosols Characterized by Field Emission Scanning Electron Microscopy (FESEM)

    PubMed Central

    Afanou, Komlavi Anani; Straumfors, Anne; Skogstad, Asbjørn; Skaar, Ida; Hjeljord, Linda; Skare, Øivind; Green, Brett James; Tronsmo, Arne; Eduard, Wijnand

    2016-01-01

    Fungal aerosols consist of spores and fragments with diverse array of morphologies; however, the size, shape, and origin of the constituents require further characterization. In this study, we characterize the profile of aerosols generated from Aspergillus fumigatus, A. versicolor, and Penicillium chrysogenum grown for 8 weeks on gypsum boards. Fungal particles were aerosolized at 12 and 20 L min−1 using the Fungal Spore Source Strength Tester (FSSST) and the Stami particle generator (SPG). Collected particles were analyzed with field emission scanning electron microscopy (FESEM). We observed spore particle fraction consisting of single spores and spore aggregates in four size categories, and a fragment fraction that contained submicronic fragments and three size categories of larger fragments. Single spores dominated the aerosols from A. fumigatus (median: 53%), while the submicronic fragment fraction was the highest in the aerosols collected from A. versicolor (median: 34%) and P. chrysogenum (median: 31%). Morphological characteristics showed near spherical particles that were only single spores, oblong particles that comprise some spore aggregates and fragments (<3.5 μm), and fiber-like particles that regroup chained spore aggregates and fragments (>3.5 μm). Further, the near spherical particles dominated the aerosols from A. fumigatus (median: 53%), while oblong particles were dominant in the aerosols from A. versicolor (68%) and P. chrysogenum (55%). Fiber-like particles represented 21% and 24% of the aerosols from A. versicolor and P. chrysogenum, respectively. This study shows that fungal particles of various size, shape, and origin are aerosolized, and supports the need to include a broader range of particle types in fungal exposure assessment. PMID:26855468

  10. Profile of heating rate due to aerosols using lidar and skyradiometer in SKYNET Hefei site

    NASA Astrophysics Data System (ADS)

    Wang, Z.; Liu, D.; Xie, C.

    2015-12-01

    Atmospheric aerosols have a significant impact on climate due to their important role in modifying atmosphere energy budget. On global scale, the direct radiative forcing is estimated to be in the range of -0.9 to -0.1 Wm-2 for aerosols [1]. Yet, these estimates are subject to very large uncertainties because of uncertainties in spatial and temporal variations of aerosols. At local scales, as aerosol properties can vary spatially and temporally, radiative forcing due to aerosols can be also very different and it can exceed the global value by an order of magnitude. Hence, it is very important to investigate aerosol loading, properties, and radiative forcing due to them in detail on local regions of climate significance. Haze and dust events in Hefei, China are explored by Lidar and Skyradiometer. Aerosol optical properties including the AOD, SSA, AAE and size distribution are analysed by using the SKYRAD.PACK [2] and presented in this paper. Furthermore, the radiative forcing due to aerosols and the heating rate in the ATM are also calculated using SBDART model [3]. The results are shown that the vertical heating rate is tightly related to aerosol profile. References: 1. IPCC. 2007. Climate Change 2007: The Physical Science Basic. Contribution of Working Group I Contribution to the Intergovernmental Panel on Climate Change Fourth Assessment Report. Solomon S, Qing D H, Manning M, et al. eds., Cambridge University Press, Cambridge, United Kingdom and New York, N Y, USA. 2. Nakajima, T., G. Tonna, R. Rao, Y. Kaufman, and B. Holben, 1996: Use of sky brightness measurements from ground for remote sensing of particulate poly dispersions, Appl. Opt., 35, 2672-2686. 3. Ricchiazzi et al 1998. SBDART: a research and teaching software tool for plane-parallel radiative transfer in the Earth's atmosphere,Bulletin of the American Meteorological Society,79,2101-2114.

  11. Vertical Profiles of Cloud Condensation Nuclei, Condensation Nuclei, Optical Aerosol, Aerosol Optical Properties, and Aerosol Volatility Measured from Balloons

    NASA Technical Reports Server (NTRS)

    Deshler, T.; Snider, J. R.; Vali, G.

    1998-01-01

    Under the support of this grant a balloon-borne gondola containing a variety of aerosol instruments was developed and flown from Laramie, Wyoming, (41 deg N, 105 deg W) and from Lauder, New Zealand (45 deg S, 170 deg E). The gondola includes instruments to measure the concentrations of condensation nuclei (CN), cloud condensation nuclei (CCN), optically detectable aerosol (OA.) (r greater than or equal to 0.15 - 2.0 microns), and optical scattering properties using a nephelometer (lambda = 530 microns). All instruments sampled from a common inlet which was heated to 40 C on ascent and to 160 C on descent. Flights with the CN counter, OA counter, and nephelometer began in July 1994. The CCN counter was added in November 1994, and the engineering problems were solved by June 1995. Since then the flights have included all four instruments, and were completed in January 1998. Altogether there were 20 flights from Laramie, approximately 5 per year, and 2 from Lauder. Of these there were one or more engineering problems on 6 of the flights from Laramie, hence the data are somewhat limited on those 6 flights, while a complete data set was obtained from the other 14 flights. Good CCN data are available from 12 of the Laramie flights. The two flights from Lauder in January 1998 were successful for all measurements. The results from these flights, and the development of the balloon-bome CCN counter have formed the basis for five conference presentations. The heated and unheated CN and OA measurements have been used to estimate the mass fraction of the aerosol volatile, while comparisons of the nephelometer measurements were used to estimate the light scattering, associated with the volatile aerosol. These estimates were calculated for 0.5 km averages of the ascent and descent data between 2.5 km and the tropopause, near 11.5 km.

  12. Ceilometer calibration for retrieval of aerosol optical properties

    NASA Astrophysics Data System (ADS)

    Jin, Yoshitaka; Kai, Kenji; Kawai, Kei; Nagai, Tomohiro; Sakai, Tetsu; Yamazaki, Akihiro; Uchiyama, Akihiro; Batdorj, Dashdondog; Sugimoto, Nobuo; Nishizawa, Tomoaki

    2015-03-01

    Ceilometers are durable compact backscatter lidars widely used to detect cloud base height. They are also useful for measuring aerosols. We introduced a ceilometer (CL51) for observing dust in a source region in Mongolia. For retrieving aerosol profiles with a backscatter lidar, the molecular backscatter signal in the aerosol free heights or system constant of the lidar is required. Although the system constant of the ceilometer is calibrated by the manufacturer, it is not necessarily accurate enough for the aerosol retrieval. We determined a correction factor, which is defined as the ratio of true attenuated backscattering coefficient to the measured attenuated backscattering coefficient, for the CL51 ceilometer using a dual-wavelength Mie-scattering lidar in Tsukuba, Japan before moving the ceilometer to Dalanzadgad, Mongolia. The correction factor determined by minimizing the difference between the ceilometer and lidar backscattering coefficients was approximately 1.2±0.1. Applying the correction to the CL51 signals, the aerosol optical depth (AOD) agreed well with the sky-radiometer AOD during the observation period (13-17 February 2013) in Tsukuba (9 ×10-3 of mean square error). After moving the ceilometer to Dalanzadgad, however, the AOD observed with the CL51 (calibrated by the correction factor determined in Tsukuba) was approximately 60% of the AErosol RObotic NETwork (AERONET) sun photometer AOD. The possible causes of the lower AOD results are as follows: (1) the limited height range of extinction integration (< 3 km); (2) change in the correction factor during the ceilometer transportation or with the window contamination in Mongolia. In both cases, on-site calibrations by dual-wavelength lidar are needed. As an alternative method, we showed that the backward inversion method was useful for retrieving extinction coefficients if the AOD was larger than 1.5. This retrieval method does not require the system constant and molecular backscatter signals

  13. The Aerosol Limb Imager: acousto-optic imaging of limb-scattered sunlight for stratospheric aerosol profiling

    NASA Astrophysics Data System (ADS)

    Elash, B. J.; Bourassa, A. E.; Loewen, P. R.; Lloyd, N. D.; Degenstein, D. A.

    2016-03-01

    The Aerosol Limb Imager (ALI) is an optical remote sensing instrument designed to image scattered sunlight from the atmospheric limb. These measurements are used to retrieve spatially resolved information of the stratospheric aerosol distribution, including spectral extinction coefficient and particle size. Here we present the design, development and test results of an ALI prototype instrument. The long-term goal of this work is the eventual realization of ALI on a satellite platform in low earth orbit, where it can provide high spatial resolution observations, both in the vertical and cross-track. The instrument design uses a large-aperture acousto-optic tunable filter (AOTF) to image the sunlit stratospheric limb in a selectable narrow wavelength band ranging from the visible to the near infrared. The ALI prototype was tested on a stratospheric balloon flight from the Canadian Space Agency (CSA) launch facility in Timmins, Canada, in September 2014. Preliminary analysis of the hyperspectral images indicates that the radiance measurements are of high quality, and we have used these to retrieve vertical profiles of stratospheric aerosol extinction coefficient from 650 to 1000 nm, along with one moment of the particle size distribution. Those preliminary results are promising and development of a satellite prototype of ALI within the Canadian Space Agency is ongoing.

  14. Comparison of Aerosol Classification from Airborne High Spectral Resolution Lidar and the CALIPSO Vertical Feature Mask

    NASA Astrophysics Data System (ADS)

    Burton, S. P.; Ferrare, R. A.; Omar, A. H.; Hostetler, C. A.; Hair, J. W.; Rogers, R.; Obland, M. D.; Butler, C. F.; Cook, A. L.; Harper, D. B.

    2012-12-01

    The NASA Langley Research Center (LaRC) airborne High Spectral Resolution Lidar (HSRL-1) on the NASA B200 aircraft has acquired large datasets of aerosol extinction (532nm), backscatter (532 and 1064nm), and depolarization (532 and 1064nm) profiles during 349 science flights in 19 field missions across North America since 2006. The extinction-to-backscatter ratio ("lidar ratio"), aerosol depolarization ratios, and backscatter color ratio measurements from HSRL-1 are scale-invariant parameters that depend on aerosol type but not concentration. These four aerosol intensive parameters are combined to qualitatively classify HSRL aerosol measurements into eight separate composition types. The classification methodology uses models formed from "training cases" with known aerosol type. The remaining measurements are then compared with these models using the Mahalanobis distance. Aerosol products from the CALIPSO satellite include aerosol type information as well, which is used as input to the CALIPSO aerosol retrieval. CALIPSO aerosol types are inferred using a mix of aerosol loading-dependent parameters, estimated aerosol depolarization, and location, altitude, and surface type information. The HSRL instrument flies beneath the CALIPSO satellite orbit track, presenting the opportunity for comparisons between the HSRL aerosol typing and the CALIPSO Vertical Feature Mask Aerosol Subtype product, giving insight into the performance of the CALIPSO aerosol type algorithm. We find that the aerosol classification from the two instruments frequently agree for marine aerosols and pure dust, and somewhat less frequently for pollution and smoke. In addition, the comparison suggests that the CALIPSO polluted dust type is overly inclusive, encompassing cases of dust combined with marine aerosol as well as cases without much evidence of dust. Qualitative classification of aerosol type combined with quantitative profile measurements of aerosol backscatter and extinction has many useful

  15. Vertical Resolved Dust Mass Concentration and Backscatter Coefficient Retrieval of Asian Dust Plume Using Quartz Raman Channel in Lidar Measurements

    NASA Astrophysics Data System (ADS)

    Noh, Young M.; Mueller, Detlef; Shin, Sungkyun

    2016-06-01

    In this work, we present a method for estimating vertical resolved mass concentration of dust immersed in Asian dust plume using Raman scattering of quartz (silicon dioxide, silica). During the Asian dust period of March 15, 16, and 21 in 2010, Raman lidar measurements detected the presence of quartz, and successfully showed the vertical profiles of the quartz backscatter coefficient. Since the Raman backscatter coefficient was connected with the Raman backscatter differential cross section and the number density of quartz molecules, the mass concentration of quartz in the atmosphere can be estimated from the quartz backscatter coefficient. The weight percentage from 40 to 70 % for quartz in the Asian dust was estimated from references. The vertical resolved mass concentration of dust was estimated by quartz mass concentration and weight percentage. We also present a retrieval method to obtain dust backscatter coefficient from the mixed Asian dust and pollutant layer. OPAC (Optical Properties of Aerosol and Clouds) simulations were conducted to calculate dust backscatter coefficient. The retrieved dust mass concentration was used as an input parameter for the OPAC calculations. These approaches in the study will be useful for characterizing the quartz dominated in the atmospheric aerosols and estimating vertical resolved mass concentration of dust. It will be especially applicable for optically distinguishing the dust and non-dust aerosols in studies on the mixing state of Asian dust plume. Additionally, the presented method combined with satellite observations is enable qualitative and quantitative monitoring for Asian dust.

  16. LASE measurements of aerosols and water vapor during TARFOX

    NASA Technical Reports Server (NTRS)

    Ferrare, Richard A.; Ismail, Syed; Browell, Edward V.; Brackett, Vincent G.; Kooi, Susan A.; Clayton, Marian B.; Melfi, Harvey; Whiteman, David N.; Schwenner, Geary; Evans, Keith D.; Hobbs, Peter V.; Veefkind, J. Pepijn; Russell, Philip B.; Livingston, John M.; Hignett, Philip; Holben, Brent N.; Remer, Lorraine A.

    1998-01-01

    The TARFOX (Tropospheric Aerosol Radiative Forcing Observational Experiment) intensive field campaign was designed to reduce uncertainties in estimates of the effects of anthropogenic aerosols on climate by measuring direct radiative effects and the optical, physical, and chemical properties of aerosols [1]. TARFOX was conducted off the East Coast of the United States between July 10-31, 1996. Ground, aircraft, and satellite-based sensors measured the sensitivity of radiative fields at various atmospheric levels to aerosol optical properties (i.e., optical thickness, phase function, single-scattering albedo) and to the vertical profile of aerosols. The LASE (Lidar Atmospheric Sensing Experiment) instrument, which was flown on the NASA ER-2 aircraft, measured vertical profiles of total scattering ratio and water vapor during a series of 9 flights. These profiles were used in real-time to help direct the other aircraft to the appropriate altitudes for intensive sampling of aerosol layers. We have subsequently used the LASE aerosol data to derive aerosol backscattering and extinction profiles. Using these aerosol extinction profiles, we derived estimates of aerosol optical thickness (AOT) and compared these with measurements of AOT from both ground and airborne sun photometers and derived from the ATSR-2 (Along Track and Scanning Radiometer 2) sensor on ERS-2 (European Remote Sensing Satellite-2). We also used the water vapor mixing ratio profiles measured simultaneously by LASE to derive precipitable water vapor and compare these to ground based measurements.

  17. Infrared backscattering

    NASA Technical Reports Server (NTRS)

    Bohren, Craig F.; Nevitt, Timothy J.; Singham, Shermila Brito

    1989-01-01

    All particles in the atmosphere are not spherical. Moreover, the scattering properties of randomly oriented nonspherical particles are not equivalent to those of spherical particles no matter how the term equivalent is defined. This is especially true for scattering in the backward direction and at the infrared wavelengths at which some atmospheric particles have strong absorption bands. Thus calculations based on Mie theory of infrared backscattering by dry or insoluble atmospheric particles are suspect. To support this assertion, it was noted that peaks in laboratory-measured infrared backscattering spectra show appreciable shifts compared with those calculated using Mie theory. One example is ammonium sulfate. Some success was had in modeling backscattering spectra of ammonium sulfate particles using a simple statistical theory called the continuous distribution of ellipsoids (CDE) theory. In this theory, the scattering properties of an ensemble are calculated. Recently a modified version of this theory was applied to measured spectra of scattering by kaolin particles. The particles were platelike, so the probability distribution of ellipsoidal shapes was chosen to reflect this. As with ammonium sulfate, the wavelength of measured peak backscattering is shifted longward of that predicted by Mie theory.

  18. A Multi-Instrument Approach for Characterizing the Vertical Structure of Aerosol Properties: Case Studies in the Pacific Basin Troposphere

    NASA Technical Reports Server (NTRS)

    Redemann, J.; Turco, R. P.; Pueschel, R. F.; Fenn, M. A.; Browell, E. V.; Grant, W. B.

    1998-01-01

    During February/March 1994, a series of aircraft-based aerosol measurements were carried out in the Pacific Basin troposphere using a differential absorption lidar system deployed by NASA Langley, and optical spectrometer probes and a wire-impactor system operated by NASA Ames. A modified Klett inversion algorithm was applied to extract altitude profiles of aerosol backscattering from the IR lidar signal. The algorithm that we have designed for this purpose utilizes the in situ aerosol measurements to normalize the lidar profile at the aircraft altitude and to supply the lidar ratio as a function of height. The lidar-derived aerosol backscattering coefficients were then compared to the backscattering coefficients calculated from the in situ measurements. During several local aircraft descents, we found good agreement between the remote lidar and in situ results for the absolute value of the aerosol backscattering coefficient and its altitude variation only when we allowed for several layers with different aerosol refractive indices. The agreement validates our lidar calibration method and provides an indication of the variation in aerosol refractive index as a function of altitude. Two of the three case studies performed in this paper reveal layers of anthropogenic aerosols transported long distances into the Pacific Basin troposphere. A third case implies the existence of a layer of dustlike aerosol particles in the lower troposphere, most likely of Asian origin.

  19. A multi-instrument approach for characterizing the vertical structure of aerosol properties: Case studies in the Pacific Basin troposphere

    NASA Astrophysics Data System (ADS)

    Redemann, J.; Turco, R. P.; Pueschel, R. F.; Fenn, M. A.; Browell, E. V.; Grant, W. B.

    1998-09-01

    During February/March 1994, a series of aircraft-based aerosol measurements were carried out in the Pacific Basin troposphere using a differential absorption lidar system deployed by NASA Langley, and optical spectrometer probes and a wire-impactor system operated by NASA Ames. A modified Klett inversion algorithm was applied to extract altitude profiles of aerosol backscattering from the IR lidar signal. The algorithm that we have designed for this purpose utilizes the in situ aerosol measurements to normalize the lidar profile at the aircraft altitude and to supply the lidar ratio as a function of height. The lidar-derived aerosol backscattering coefficients were then compared to the backscattering coefficients calculated from the in situ measurements. During several local aircraft descents, we found good agreement between the remote lidar and in situ results for the absolute value of the aerosol backscattering coefficient and its altitude variation only when we allowed for several layers with different aerosol refractive indices. The agreement validates our lidar calibration method and provides an indication of the variation in aerosol refractive index as a function of altitude. Two of the three case studies performed in this paper reveal layers of anthropogenic aerosols transported long distances into the Pacific Basin troposphere. A third case implies the existence of a layer of dustlike aerosol particles in the lower troposphere, most likely of Asian origin.

  20. Atmospheric Backscatter Model Development for CO Sub 2 Wavelengths

    NASA Technical Reports Server (NTRS)

    Deepak, A.; Kent, G.; Yue, G. K.

    1982-01-01

    The results of investigations into the problems of modeling atmospheric backscatter from aerosols, in the lowest 20 km of the atmosphere, at CO2 wavelengths are presented, along with a summary of the relevant aerosol characteristics and their variability, and a discussion of the measurement techniques and errors involved. The different methods of calculating the aerosol backscattering function, both from measured aerosol characteristics and from optical measurements made at other wavelengths, are discussed in detail, and limits are placed on the accuracy of these methods. The effects of changing atmospheric humidity and temperature on the backscatter are analyzed and related to the actual atmosphere. Finally, the results of modeling CO2 backscatter in the atmosphere are presented and the variation with height and geographic location discussed, and limits placed on the magnitude of the backscattering function. Conclusions regarding modeling techniques and modeled atmospheric backscatter values are presented in tabular form.

  1. Autonomous Ozone and Aerosol LIDAR Profiling of the Troposphere: A Synergistic Approach

    NASA Astrophysics Data System (ADS)

    Strawbridge, K. B.

    2015-12-01

    LIDAR technology is an excellent tool to probe the complex vertical structure of the atmosphere at high spatial and temporal resolution. This provides the critical vertical context for the interpretation of ground-based chemistry measurements, airborne measurements and model/satellite verification and validation. In recent years, Environment Canada has designed several autonomous aerosol LIDAR systems for deployment across several regions of Canada. The current system builds on the successes of these autonomous LIDARS but using a synergistic approach by combining tropospheric ozone DIAL (Differential Absorption LIDAR) technology with simultaneous 3+2+1 aerosol LIDAR measurements. It operates 24 hours a day, seven days a week except during precipitation events. The system is operated remotely and the data are updated every hour to a website to allow near real-time capability. A few case studies are shown emphasizing the synergistic approach of coupling ozone and aerosol profiles to better understand air quality impacts on local and regional scales.

  2. Light scattering characteristics of various aerosol types derived from multiple wavelength lidar observations.

    PubMed

    Sasano, Y; Browell, E V

    1989-05-01

    The present study demonstrates the potential of a multiple wavelength lidar for discriminating between several aerosol types such as maritime, continental, stratospheric, and desert aerosols on the basis of wavelength dependence of the aerosol backscatter coefficient. In the analysis of lidar signals, the two-component lidar equation was solved under the assumption of similarity in the derived profiles of backscatter coefficients for each wavelength, and this made it possible to reduce the uncertainty in the extinction/backscatter ratio, which is a key parameter in the lidar solution. It is shown that a three-wavelength lidar system operating at 300, 600, and 1064 nm can provide unique information for discriminating between various aerosol types such as continental, maritime, Saharan dust, stratospheric aerosols in a tropopause fold event, and tropical forest aerosols. Measurement error estimation was also made through numerical simulations. Mie calculations were made using in situ aerosol data and aerosol models to compare with the lidar results. There was disagreement between the theoretical and empirical results, which in some cases was substantial. These differences may be partly due to uncertainties in the lidar data analysis and aerosol characteristics and also due to the conventional assumption of aerosol sphericity for the aerosol Mie calculations. PMID:20548724

  3. Balloonborne measurements of ozone and aerosol profiles at McMurdo Station, Antarctica, during the austral spring of 1992

    SciTech Connect

    Johnson, B.J.; Deshler, T. )

    1993-01-01

    This paper reports some of the findings of an overall study of the ozone hole over Antarctica. Vertical profiles of ozone and aerosols were measured, and the inclusion of aerosols from the June 1991 eruption of Mount Pinatubo was of particular interest. 4 refs., 2 figs.

  4. A sensitivity study on the retrieval of aerosol vertical profiles using the oxygen A-band

    NASA Astrophysics Data System (ADS)

    Colosimo, S. F.; Natraj, V.; Sander, S. P.; Stutz, J.

    2015-11-01

    Atmospheric absorption in the O2 A-band (12 950-13 200 cm-1) offers a unique opportunity to retrieve aerosol extinction profiles from space-borne measurements due to the large dynamic range of optical thickness in that spectral region. Absorptions in strong O2 lines are saturated; therefore, any radiance measured in these lines originates from scattering in the upper part of the atmosphere. Outside of O2 lines, or in weak lines, the atmospheric column absorption is small, and light penetrates to lower atmospheric layers, allowing for the quantification of aerosols and other scatterers near the surface. While the principle of aerosol profile retrieval using O2 A-band absorption from space is well known, a thorough quantification of the information content, i.e., the amount of vertical profile information that can be obtained, and the dependence of the information content on the spectral resolution of the measurements, has not been thoroughly conducted. Here, we use the linearized vector radiative transfer model VLIDORT to perform spectrally resolved simulations of atmospheric radiation in the O2 A-band in the presence of aerosol for four different generic scenarios: Urban, Highly polluted, Elevated layer, and Marine-Arctic. The high-resolution radiances emerging from the top of the atmosphere are degraded to different spectral resolutions, simulating spectrometers with different resolving powers. We use optimal estimation theory to quantify the information content in the aerosol profile retrieval with respect to different aerosol parameters and instrument spectral resolutions. The simulations show that better spectral resolution generally leads to an increase in the total amount of information that can be retrieved, with the number of degrees of freedom (DoF) varying between 0.34-2.11 at low resolution (5 cm-1) to 3.43-5.92 at high resolution (0.05 cm-1) for the four different cases. A particularly strong improvement was found in the retrieval of tropospheric

  5. Initial Verification of GEOS-4 Aerosols Using CALIPSO and MODIS: Scene Classification

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth J.; Colarco, Peter R.; Hlavka, Dennis; Levy, Robert C.; Vaughan, Mark A.; daSilva, Arlindo

    2007-01-01

    A-train sensors such as MODIS and MISR provide column aerosol properties, and in the process a means of estimating aerosol type (e.g. smoke vs. dust). Correct classification of aerosol type is important because retrievals are often dependent upon selection of the right aerosol model. In addition, aerosol scene classification helps place the retrieved products in context for comparisons and analysis with aerosol transport models. The recent addition of CALIPSO to the A-train now provides a means of classifying aerosol distribution with altitude. CALIPSO level 1 products include profiles of attenuated backscatter at 532 and 1064 nm, and depolarization at 532 nm. Backscatter intensity, wavelength ratio, and depolarization provide information on the vertical profile of aerosol concentration, size, and shape. Thus similar estimates of aerosol type using MODIS or MISR are possible with CALIPSO, and the combination of data from all sensors provides a means of 3D aerosol scene classification. The NASA Goddard Earth Observing System general circulation model and data assimilation system (GEOS-4) provides global 3D aerosol mass for sulfate, sea salt, dust, and black and organic carbon. A GEOS-4 aerosol scene classification algorithm has been developed to provide estimates of aerosol mixtures along the flight track for NASA's Geoscience Laser Altimeter System (GLAS) satellite lidar. GLAS launched in 2003 and did not have the benefit of depolarization measurements or other sensors from the A-train. Aerosol typing from GLAS data alone was not possible, and the GEOS-4 aerosol classifier has been used to identify aerosol type and improve the retrieval of GLAS products. Here we compare 3D aerosol scene classification using CALIPSO and MODIS with the GEOS-4 aerosol classifier. Dust, smoke, and pollution examples will be discussed in the context of providing an initial verification of the 3D GEOS-4 aerosol products. Prior model verification has only been attempted with surface mass

  6. Vertical profiling of aerosol hygroscopic properties in the planetary boundary layer during the PEGASOS campaigns

    NASA Astrophysics Data System (ADS)

    Rosati, Bernadette; Gysel, Martin; Rubach, Florian; Mentel, Thomas F.; Goger, Brigitta; Poulain, Laurent; Schlag, Patrick; Miettinen, Pasi; Pajunoja, Aki; Virtanen, Annele; Klein Baltink, Henk; Bas Henzing, J. S.; Größ, Johannes; Gobbi, Gian Paolo; Wiedensohler, Alfred; Kiendler-Scharr, Astrid; Decesari, Stefano; Facchini, Maria Cristina; Weingartner, Ernest; Baltensperger, Urs

    2016-06-01

    Vertical profiles of the aerosol particles hygroscopic properties, their mixing state as well as chemical composition were measured above northern Italy and the Netherlands. An aerosol mass spectrometer (AMS; for chemical composition) and a white-light humidified optical particle spectrometer (WHOPS; for hygroscopic growth) were deployed on a Zeppelin NT airship within the PEGASOS project. This allowed one to investigate the development of the different layers within the planetary boundary layer (PBL), providing a unique in situ data set for airborne aerosol particles properties in the first kilometre of the atmosphere. Profiles measured during the morning hours on 20 June 2012 in the Po Valley, Italy, showed an increased nitrate fraction at ˜ 100 m above ground level (a.g.l.) coupled with enhanced hygroscopic growth compared to ˜ 700 m a. g. l. This result was derived from both measurements of the aerosol composition and direct measurements of the hygroscopicity, yielding hygroscopicity parameters (κ) of 0.34 ± 0.12 and 0.19 ± 0.07 for 500 nm particles, at ˜ 100 and ˜ 700 m a. g. l., respectively. The difference is attributed to the structure of the PBL at this time of day which featured several independent sub-layers with different types of aerosols. Later in the day the vertical structures disappeared due to the mixing of the layers and similar aerosol particle properties were found at all probed altitudes (mean κ ≈ 0.18 ± 0.07). The aerosol properties observed at the lowest flight level (100 m a. g. l.) were consistent with parallel measurements at a ground site, both in the morning and afternoon. Overall, the aerosol particles were found to be externally mixed, with a prevailing hygroscopic fraction. The flights near Cabauw in the Netherlands in the fully mixed PBL did not feature altitude-dependent characteristics. Particles were also externally mixed and had an even larger hygroscopic fraction compared to the results in Italy. The mean κ from

  7. CALIOP near-real-time backscatter products compared to EARLINET data

    NASA Astrophysics Data System (ADS)

    Grigas, T.; Hervo, M.; Gimmestad, G.; Forrister, H.; Schneider, P.; Preißler, J.; Tarrason, L.; O'Dowd, C.

    2015-03-01

    The expedited near-real-time Level 1.5 Cloud-Aerosol Lidar (Light Detection and Ranging) with Orthogonal Polarization (CALIOP) products were evaluated against data from the ground-based European Aerosol Research Lidar Network (EARLINET). Over a period of three years, lidar data from 48 CALIOP overpasses with ground tracks within a 100 km distance from an operating EARLINET station were deemed suitable for analysis and they included a valid aerosol classification type (e.g. dust, polluted dust, clean marine, clean continental, polluted continental, mixed and/or smoke/biomass burning). For the complete dataset comprising both PBL and FT data, the correlation coefficient was 0.86, and when separated into separate layers, the PBL and FT correlation coefficients were 0.6 and 0.85 respectively. The presence of FT layers with high attenuated backscatter led to poor agreement in PBL backscatter profiles between the CALIOP and EARLINET measurements and prompted a further analysis filtering out such cases. However, the correlation coefficient value for the complete dataset decreased marginally from 0.86 to 0.84 while the PBL coefficient increased from 0.6 up to 0.65 and the FT coefficient also decreased from 0.85 to 0.79. For specific aerosol types, the correlation coefficient between CALIOP backscatter profiles and ground-based lidar data ranged from 0.37 for polluted continental aerosol in the planetary boundary layer (PBL) to 0.57 for dust in the free troposphere (FT). The results suggest different levels of agreement based on the location of the dominant aerosol layer and the aerosol type.

  8. Variability in Vertical Profiles of Water Vapor Associated with African Aerosol over the Tropical Atlantic

    NASA Astrophysics Data System (ADS)

    Huang, J.; Zhang, C.; Prospero, J. M.

    2007-12-01

    We used four years (2003-2006) of MODIS aerosol optical depth and concurrent AIRS profiled water vapor to explore how the vertical distribution of water vapor may systematically change with outbreaks of African aerosol over the tropical Atlantic Ocean. The first step was to look for a relationship in the Barbados region using in-situ Barbados dust record and the profiled relative humidity from meteorological soundings. We extended the study to the synoptic scale in the West Indies using the MODIS and AIRS products. In the tropical Atlantic, preliminary results indicate that water vapor at 850-1000 hPa is significantly less in July on dusty days than clean days over the northeastern tropical Atlantic [5-25N, 30-20W] where African dust is predominant. In contrast, over the southeastern tropical Atlantic [15S-0, 5W-10E], where African biomass burning smoke prevails, water vapor at 600-1000 hPa is significantly higher in August on smoky days than clean days. Additionally, in January when African mixed aerosol (dust and smoke) is anomalously high over the equatorial eastern tropical Atlantic [5S-5N, 15W-5E], less water vapor is observed at two levels: 925-1000 hPa and 500-600 hPa. It is hypothesized that these results are associated with the non-hygroscopic nature of African dust, the hygroscopic properties of African smoke, and their transport pathways over the tropical Atlantic. These results are useful in the design and diagnostics of model simulations of climate effects of aerosols such as aerosol related precipitation change.

  9. Utilizing The Synergy of Airborne Backscatter Lidar and In-Situ Measurements for Evaluating CALIPSO

    NASA Astrophysics Data System (ADS)

    Tsekeri, Alexandra; Amiridis, Vassilis; Marenco, Franco; Marinou, Eleni; Rosenberg, Phil; Solomos, Stavros; Trembath, Jamie; Allan, James; Bacak, Asan; Nenes, Athanasios

    2016-06-01

    Airborne campaigns dedicated to satellite validation are crucial for the effective global aerosol monitoring. CALIPSO is currently the only active remote sensing satellite mission, acquiring the vertical profiles of the aerosol backscatter and extinction coefficients. Here we present a method for CALIPSO evaluation from combining lidar and in-situ airborne measurements. The limitations of the method have to do mainly with the in-situ instrumentation capabilities and the hydration modelling. We also discuss the future implementation of our method in the ICE-D campaign (Cape Verde, August 2015).

  10. Statistical Characteristics of Aerosol Extinction Coefficient Profile in East Asia from CALIPSO

    NASA Astrophysics Data System (ADS)

    Sun, Xuejin; Zhou, Junhao; Zhou, Yongbo

    2016-06-01

    Aerosol extinction coefficient profile (ECP) is important in radiative transfer modeling, however, knowledge of ECP in some area has not been clearly recognized. To get a full understanding of statistical characteristics of ECP in three Asian regions: the Mongolian Plateau, the North China Plain and the Yellow Sea, CALIPSO aerosol product in 2012 is processed by conventional statistical methods. Orbit averaged ECP turns out to be mainly exponential and Gaussian patterns. Curve fitting shows that the two ECP patterns account for more than 50 percent of all the samples, especially in the Yellow Sea where the frequency of occurrence even reaches over 80 percent. Parameters determining fitting curves are provided consequently. To be specific, Gaussian pattern is the main ECP distribution in the Mongolian Plateau and the Yellow Sea, and exponential pattern predominates in the North China Plain. Besides, aerosol scale height reaches its maximum in summer and in the Mongolian Plateau. Meanwhile, the uplifting and deposition of dust during transportation are potentially explanations to the occurrence of Gaussian ECP. The results have certain representativeness, and contribute to reducing uncertainties of aerosol model in relevant researches.

  11. Single-Particle Black Carbon Aerosol Verticle Profiles From the Boundary Layer to the Lower Stratosphere

    NASA Astrophysics Data System (ADS)

    Schwarz, J. P.; Gao, R. S.; Fahey, D. W.; Laurel, W. A.; Thomson, D. S.; Kok, G. L.; Baumgardner, D.; Wilson, J. C.; Lopez, J.; Aikin, K.; Jost, H.; Thompson, T. L.; Reeves, J. M.; Lowenstein, M.

    2005-12-01

    A single-particle soot photometer (SP2) was flown on a NASA WB-57F high-altitude research aircraft in November 2004 from Houston, TX. The SP2 uses laser-induced incandescence to directly measure the mass of individual black-carbon (BC) particles in the mass range of ~0.3-300 fg. Scattered light is used to size non-absorbing aerosols in the range of ~150 - 700 nm diameter. Data from two mid-latitude flights has been used to generate size distributions and profiles of both aerosol types from the boundary layer to the lower stratosphere. Results for scattering aerosol concentrations are in good agreement with typical particle spectrometer measurements in the same region. Mass mixing ratios of BC between 5 and 18.7 km were roughly an order of magnitude lower than typical values as reported with wire impactor measurements and as predicted by two global BC models. The impact of this discrepancy on estimates of direct radiative forcing of BC aerosol will also be discussed.

  12. Estimation of surface-level PM concentration from satellite observation taking into account the aerosol vertical profiles and hygroscopicity.

    PubMed

    Kim, Kwanchul; Lee, Kwon H; Kim, Ji I; Noh, Youngmin; Shin, Dong H; Shin, Sung K; Lee, Dasom; Kim, Jhoon; Kim, Young J; Song, Chul H

    2016-01-01

    Surface-level PM10 distribution was estimated from the satellite aerosol optical depth (AOD) products, taking the account of vertical profiles and hygroscopicity of aerosols over Jeju, Korea during March 2008 and October 2009. In this study, MODIS AOD data from the Terra and Aqua satellites were corrected with aerosol extinction profiles and relative humidity data. PBLH (Planetary Boundary Layer Height) was determined from MPLNET lidar-derived aerosol extinction coefficient profiles. Through statistical analysis, better agreement in correlation (R = 0.82) between the hourly PM10 concentration and hourly average Sunphotometer AOD was the obtained when vertical fraction method (VFM) considering Haze Layer Height (HLH) and hygroscopic growth factor f(RH) was used. The validity of the derived relationship between satellite AOD and surface PM10 concentration clearly demonstrates that satellite AOD data can be utilized for remote sensing of spatial distribution of regional PM10 concentration. PMID:26421659

  13. Estimation of surface-level PM concentration from satellite observation taking into account the aerosol vertical profiles and hygroscopicity.

    PubMed

    Kim, Kwanchul; Lee, Kwon H; Kim, Ji I; Noh, Youngmin; Shin, Dong H; Shin, Sung K; Lee, Dasom; Kim, Jhoon; Kim, Young J; Song, Chul H

    2016-01-01

    Surface-level PM10 distribution was estimated from the satellite aerosol optical depth (AOD) products, taking the account of vertical profiles and hygroscopicity of aerosols over Jeju, Korea during March 2008 and October 2009. In this study, MODIS AOD data from the Terra and Aqua satellites were corrected with aerosol extinction profiles and relative humidity data. PBLH (Planetary Boundary Layer Height) was determined from MPLNET lidar-derived aerosol extinction coefficient profiles. Through statistical analysis, better agreement in correlation (R = 0.82) between the hourly PM10 concentration and hourly average Sunphotometer AOD was the obtained when vertical fraction method (VFM) considering Haze Layer Height (HLH) and hygroscopic growth factor f(RH) was used. The validity of the derived relationship between satellite AOD and surface PM10 concentration clearly demonstrates that satellite AOD data can be utilized for remote sensing of spatial distribution of regional PM10 concentration.

  14. CALIOP near-real-time backscatter products compared to EARLINET data

    NASA Astrophysics Data System (ADS)

    Grigas, T.; Hervo, M.; Gimmestad, G.; Forrister, H.; Schneider, P.; Preißler, J.; Tarrason, L.; O'Dowd, C.

    2015-11-01

    The expedited near-real-time Level 1.5 Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) version 3 products were evaluated against data from the ground-based European Aerosol Research Lidar Network (EARLINET). The statistical framework and results of the three-year evaluation of 48 CALIOP overpasses with ground tracks within a 100 km distance from operating EARLINET stations are presented and include analysis for the following CALIOP classifications of aerosol type: dust, polluted dust, clean marine, clean continental, polluted continental, mixed and/or smoke/biomass burning. For the complete data set comprising both the planetary boundary layer (PBL) and the free troposphere (FT) data, the correlation coefficient (R) was 0.86. When the analysis was conducted separately for the PBL and FT, the correlation coefficients were R = 0.6 and R = 0.85, respectively. From analysis of selected specific cases, it was initially thought that the presence of FT layers, with high attenuated backscatter, led to poor agreement of the PBL backscatter profiles between the CALIOP and EARLINET and prompted a further analysis to filter out such cases; however, removal of these layers did not improve the agreement as R reduced marginally from R = 0.86 to R = 0.84 for the combined PBL and FT analysis, increased marginally from R = 0.6 up to R = 0.65 for the PBL on its own, and decreased marginally from R = 0.85 to R = 0.79 for the FT analysis on its own. This suggests considerable variability, across the data set, in the spatial distribution of the aerosol over spatial scales of 100 km or less around some EARLINET stations rather than influence from elevated FT layers. For specific aerosol types, the correlation coefficient between CALIOP backscatter profiles and the EARLINET data ranged from R = 0.37 for polluted continental aerosol in the PBL to R = 0.57 for dust in the FT.

  15. A sensitivity study on the retrieval of aerosol vertical profiles using the oxygen A-band

    NASA Astrophysics Data System (ADS)

    Fedele Colosimo, Santo; Natraj, Vijay; Sander, Stanley P.; Stutz, Jochen

    2016-04-01

    Atmospheric absorption in the O2 A-band (12 950-13 200 cm-1) offers a unique opportunity to retrieve aerosol extinction profiles from space-borne measurements due to the large dynamic range of optical thickness in that spectral region. Absorptions in strong O2 lines are saturated; therefore, any radiance measured in these lines originates from scattering in the upper part of the atmosphere. Outside of O2 lines, or in weak lines, the atmospheric column absorption is small, and light penetrates to lower atmospheric layers, allowing for the quantification of aerosols and other scatterers near the surface.

    While the principle of aerosol profile retrieval using O2 A-band absorption from space is well-known, a thorough quantification of the information content, i.e., the amount of vertical profile information that can be obtained, and the dependence of the information content on the spectral resolution of the measurements, has not been thoroughly conducted. Here, we use the linearized vector radiative transfer model VLIDORT to perform spectrally resolved simulations of atmospheric radiation in the O2 A-band for four different aerosol extinction profile scenarios: urban (urban-rural areas), highly polluted (megacity areas with large aerosol extinction), elevated layer (identifying elevated plumes, for example for biomass burning) and low extinction (representative of small aerosol extinction, such as vegetated, marine and arctic areas). The high-resolution radiances emerging from the top of the atmosphere measurements are degraded to different spectral resolutions, simulating spectrometers with different resolving powers. We use optimal estimation theory to quantify the information content in the aerosol profile retrieval with respect to different aerosol parameters and instrument spectral resolutions. The simulations show that better spectral resolution generally leads to an increase in the total amount of information that can be retrieved, with the number of

  16. Altitude profile of aerosols on Mars from measurements of its thermal radiation on limb

    NASA Technical Reports Server (NTRS)

    Moroz, V. I.; Titov, D. V.; Gektin, Yu. M.; Naraeva, M. K.; Selivanov, A. S.

    1993-01-01

    Measurements of the thermal (range 7 - 13 micrometers) radiation of Mars with the high space resolution (approximately 2 km) were made by the TERMOSKAN experiment of the Phobos mission. Some of the results were published earlier but only the surface radiation was analyzed in detail. However some part of these measurements was made near the limb of the planet. The atmosphere gives an important input here in the planetary thermal radiation. Beyond the limb the atmosphere is the only source. The task of this work is to estimate some characteristics of the atmosphere using brightness profiles of the thermal radiation near the limb. An appropriate model of the temperature profile T(h) is necessary for such an analysis. A set of T(h) models (nominal, maximal and minimal) was defined using various sources including MARSGRAM, Viking-1 lander data, its theoretical considerations and boundary layer models. On the next step the possible input of the atmospheric gaseous emissions (wing of CO2 15 micrometer band) was estimated. It was found that even for the maximal T(h) this input is no more than a few percents of the measured radiation beyond the limb. Consequently the aerosols are responsible for almost all measured emission. The analysis of the observed profile showed that these aerosols have two components: (1) exponential with the scale height about 10 km and (2) some layered structure (two layers with maxima about 23 and 33 km consisted probably of ice).

  17. The GAW Aerosol Lidar Observation Network (GALION) as a source of near-real time aerosol profile data for model evaluation and assimilation

    NASA Astrophysics Data System (ADS)

    Hoff, R. M.; Pappalardo, G.

    2010-12-01

    In 2007, the WMO Global Atmospheric Watch’s Science Advisory Group on Aerosols described a global network of lidar networks called GAW Aerosol Lidar Observation Network (GALION). GALION has a purpose of providing expanded coverage of aerosol observations for climate and air quality use. Comprised of networks in Asia (AD-NET), Europe (EARLINET and CIS-LINET), North America (CREST and CORALNET), South America (ALINE) and with contribution from global networks such as MPLNET and NDACC, the collaboration provides a unique capability to define aerosol profiles in the vertical. GALION is designed to supplement existing ground-based and column profiling (AERONET, PHOTONS, SKYNET, GAWPFR) stations. In September 2010, GALION held its second workshop and one component of discussion focussed how the network would integrate into model needs. GALION partners have contributed to the Sand and Dust Storm Warning and Analysis System (SDS-WAS) and to assimilation in models such as DREAM. This paper will present the conclusions of those discussions and how these observations can fit into a global model analysis framework. Questions of availability, latency, and aerosol parameters that might be ingested into models will be discussed. An example of where EARLINET and GALION have contributed in near-real time observations was the suite of measurements during the Eyjafjallajokull eruption in Iceland and its impact on European air travel. Lessons learned from this experience will be discussed.

  18. Retrieving the Vertical Structure of the Effective Aerosol Complex Index of Refraction from a Combination of Aerosol in Situ and Remote Sensing Measurements During TARFOX

    NASA Technical Reports Server (NTRS)

    Redemann, J.; Turco, R. P.; Liou, K. N.; Russell, P. B.; Bergstrom, R. W.; Schmid, B.; Livingston, J. M.; Hobbs, P. V.; Hartley, W. S.; Ismail, S.; Ferrare, R. A.; Browell, E. V.

    2000-01-01

    The largest uncertainty in estimates of the effects of atmospheric aerosols on climate stems from uncertainties in the determination of their microphysical properties, including the aerosol complex index of refraction, which in turn determines their optical properties. A novel technique is used to estimate the aerosol complex index of refraction in distinct vertical layers from a combination of aerosol in situ size distribution and remote sensing measurements during the Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX). In particular, aerosol backscatter measurements using the NASA Langley LASE (Lidar Atmospheric Sensing Experiment) instrument and in situ aerosol size distribution data are utilized to derive vertical profiles of the "effective" aerosol complex index of refraction at 815 nm (i.e., the refractive index that would provide the same backscatter signal in a forward calculation on the basis of the measured in situ particle size distributions for homogeneous, spherical aerosols). A sensitivity study shows that this method yields small errors in the retrieved aerosol refractive indices, provided the errors in the lidar-derived aerosol backscatter are less than 30% and random in nature. Absolute errors in the estimated aerosol refractive indices are generally less than 0.04 for the real part and can be as much as 0.042 for the imaginary part in the case of a 30% error in the lidar-derived aerosol backscatter. The measurements of aerosol optical depth from the NASA Ames Airborne Tracking Sunphotometer (AATS-6) are successfully incorporated into the new technique and help constrain the retrieved aerosol refractive indices. An application of the technique to two TARFOX case studies yields the occurrence of vertical layers of distinct aerosol refractive indices. Values of the estimated complex aerosol refractive index range from 1.33 to 1.45 for the real part and 0.001 to 0.008 for the imaginary part. The methodology devised in this study

  19. The potential of LIRIC to validate the vertical profiles of the aerosol mass concentration estimated by an air quality model

    NASA Astrophysics Data System (ADS)

    Siomos, Nikolaos; Filoglou, Maria; Poupkou, Anastasia; Liora, Natalia; Dimopoulos, Spyros; Melas, Dimitris; Chaikovsky, Anatoli; Balis, Dimitris

    2015-04-01

    Vertical profiles of the aerosol mass concentration derived by a retrieval algorithm that uses combined sunphotometer and LIDAR data (LIRIC) were used in order to validate the mass concentration profiles estimated by the air quality model CAMx. LIDAR and CIMEL measurements of the Laboratory of Atmospheric Physics of the Aristotle University of Thessaloniki were used for this validation.The aerosol mass concentration profiles of the fine and coarse mode derived by CAMx were compared with the respective profiles derived by the retrieval algorithm. For the coarse mode particles, forecasts of the Saharan dust transportation model BSC-DREAM8bV2 were also taken into account. Each of the retrieval algorithm's profiles were matched to the models' profile with the best agreement within a time window of four hours before and after the central measurement. OPAC, a software than can provide optical properties of aerosol mixtures, was also employed in order to calculate the angstrom exponent and the lidar ratio values for 355nm and 532nm for each of the model's profiles aiming in a comparison with the angstrom exponent and the lidar ratio values derived by the retrieval algorithm for each measurement. The comparisons between the fine mode aerosol concentration profiles resulted in a good agreement between CAMx and the retrieval algorithm, with the vertical mean bias error never exceeding 7 μgr/m3. Concerning the aerosol coarse mode concentration profiles both CAMx and BSC-DREAM8bV2 values are severely underestimated, although, in cases of Saharan dust transportation events there is an agreement between the profiles of BSC-DREAM8bV2 model and the retrieval algorithm.

  20. Vertical Profiles of Aerosol Particle Sizes using MGS/TES and MRO/MCS

    NASA Astrophysics Data System (ADS)

    Wolff, M. J.; Clancy, R. T.; Smith, M. D.; Benson, J. L.; McConnochie, T. H.; Pankine, A.

    2012-12-01

    Vertical variations in aerosol particle sizes often have a dramatic impact on the state and evolution of the Martian atmosphere. Recent analyses of data from the Spectroscopy for the Investigation of the Characteristics of the Atmosphere of Mars (SPICAM), the Thermal Emission Spectrometer (TES), and the Mars Climate Sounder (MCS) instruments offer some long overdue progress in constraining this aspect of aerosols. However, significantly more work remains to be done along these lines in order to better constrain and inform modern dynamical simulations of the Martian atmosphere. Thus, the primary goal of our work is to perform retrievals of particle size as a function of altitude for both dust and water ice aerosols. The choice of the TES and MCS dataset, with pole-to-pole coverage over a period of nearly eight martian years, provides the crucial systematic temporal and spatial sampling. Our presentation will include: 1) A summary of our limb radiative transfer algorithms and retrieval schemes; 2) The initial results of the application of our particle size retrieval scheme to the 2001 TES and 2007 MCS observations of those planet encircling dust events; 3) Near-term plans for for additional retrievals (aphelion cloud season, lower optical depth locations and seasons, etc.); 4) Location of the archive to be used for the distribution of the derived profiles and associated retrieval metadata.

  1. Vertical profiles of aerosol optical properties and the solar heating rate estimated by combining sky radiometer and lidar measurements

    NASA Astrophysics Data System (ADS)

    Kudo, Rei; Nishizawa, Tomoaki; Aoyagi, Toshinori

    2016-07-01

    The SKYLIDAR algorithm was developed to estimate vertical profiles of aerosol optical properties from sky radiometer (SKYNET) and lidar (AD-Net) measurements. The solar heating rate was also estimated from the SKYLIDAR retrievals. The algorithm consists of two retrieval steps: (1) columnar properties are retrieved from the sky radiometer measurements and the vertically mean depolarization ratio obtained from the lidar measurements and (2) vertical profiles are retrieved from the lidar measurements and the results of the first step. The derived parameters are the vertical profiles of the size distribution, refractive index (real and imaginary parts), extinction coefficient, single-scattering albedo, and asymmetry factor. Sensitivity tests were conducted by applying the SKYLIDAR algorithm to the simulated sky radiometer and lidar data for vertical profiles of three different aerosols, continental average, transported dust, and pollution aerosols. The vertical profiles of the size distribution, extinction coefficient, and asymmetry factor were well estimated in all cases. The vertical profiles of the refractive index and single-scattering albedo of transported dust, but not those of transported pollution aerosol, were well estimated. To demonstrate the performance and validity of the SKYLIDAR algorithm, we applied the SKYLIDAR algorithm to the actual measurements at Tsukuba, Japan. The detailed vertical structures of the aerosol optical properties and solar heating rate of transported dust and smoke were investigated. Examination of the relationship between the solar heating rate and the aerosol optical properties showed that the vertical profile of the asymmetry factor played an important role in creating vertical variation in the solar heating rate. We then compared the columnar optical properties retrieved with the SKYLIDAR algorithm to those produced with the more established scheme SKYRAD.PACK, and the surface solar irradiance calculated from the SKYLIDAR

  2. Relating Aerosol Profile and Column Measurements to Surface Concentrations: What Have We Learned from Discover-AQ?

    NASA Astrophysics Data System (ADS)

    Hoff, R. M.

    2014-12-01

    One research goal of the Deriving Information on Surface Conditions from COlumn and VERtically Resolved Observations Relevant to Air Quality (DISCOVER-AQ) mission was to determine sufficient column profile measurements to relate column integrated quantities such as Aerosol Optical Depth to surface concentrations. I will review the relationship between AOD and PM2.5 at the surface. DISCOVER-AQ in Baltimore, the San Joaquin Valley, Houston and Denver revealed quite different conditions for determining this relationship. In each case, the surface reflectivity made determination of aerosol optical depth challenging, but upward looking columns of aerosol optical depth from sunphotometers provided confirmation of the AOD results from space. In Baltimore, AOD fields reflected PM2.5 concentrations well. In California, however, the low boundary layer heights and dominance of nitrate and organic aerosols made the AOD fields less predictive of PM2.5. In California and Colorado, hydration of the aerosol varied dramatically with aerosol type (especially smoke and dust) and revealed that without an understanding of the degree of aerosol hydration with aerosol composition, the relationship between AOD and PM2.5 will continue to be a challenge. Model predictions in the Baltimore-Washington study are relatively disappointing in helping define the needed physics between the optical and microphysical properties. An overview of the measurements from DISCOVER-AQ which will help define the needed information in a more general case in the future will be given.

  3. Retrieving the Vertical Structure of the Effective Aerosol Complex Index of Refraction from a Combination of Aerosol in Situ and Remote Sensing Measurements During TARFOX

    NASA Technical Reports Server (NTRS)

    Redemann, J.; Turco, R. P.; Liou, K. N.; Russell, P. B.; Bergstrom, R. W.; Schmid, B.; Livingston, J. M.; Hobbs, P. V.; Hartley, W. S.; Ismail, S.

    2000-01-01

    The largest uncertainty in estimates of the effects of atmospheric aerosols on climate stems from uncertainties in the determination of their microphysical properties, including the aerosol complex index of refraction, which in turn determines their optical properties. A novel technique is used to estimate the aerosol complex index of refraction in distinct vertical layers from a combination of aerosol in situ size distribution and remote sensing measurements during the Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX). In particular, aerosol backscatter measurements using the NASA Langley LASE (Lidar Atmospheric Sensing Experiment) instrument and in situ aerosol size distribution data are utilized to derive vertical profiles of the 'effective' aerosol complex index of refraction at 815 nm (i.e., the refractive index that would provide the same backscatter signal in a forward calculation on the basis of the measured in situ particle size distributions for homogeneous, spherical aerosols). A sensitivity study shows that this method yields small errors in the retrieved aerosol refractive indices, provided the errors in the lidar derived aerosol backscatter are less than 30% and random in nature. Absolute errors in the estimated aerosol refractive indices are generally less than 0.04 for the real part and can be as much as 0.042 for the imaginary part in the case of a 30% error in the lidar-derived aerosol backscatter. The measurements of aerosol optical depth from the NASA Ames Airborne Tracking Sunphotometer (AATS-6) are successfully incorporated into the new technique and help constrain the retrieved aerosol refractive indices. An application of the technique to two TARFOX case studies yields the occurrence of vertical layers of distinct aerosol refractive indices. Values of the estimated complex aerosol refractive index range from 1.33 to 1.45 for the real part and 0.001 to 0.008 for the imaginary part. The methodology devised in this study

  4. Turn-key Raman lidar for profiling atmospheric water vapor, clouds, and aerosols.

    PubMed

    Goldsmith, J E; Blair, F H; Bisson, S E; Turner, D D

    1998-07-20

    We describe an operational, self-contained, fully autonomous Raman lidar system that has been developed for unattended, around-the-clock atmospheric profiling of water vapor, aerosols, and clouds. During a 1996 three-week intensive observational period, the system operated during all periods of good weather (339 out of 504 h), including one continuous five-day period. The system is based on a dual-field-of-view design that provides excellent daytime capability without sacrificing nighttime performance. It is fully computer automated and runs unattended following a simple, brief (~5-min) start-up period. We discuss the theory and design of the system and present detailed analyses of the derivation of water-vapor profiles from the lidar measurements. PMID:18285967

  5. Turn-key Raman lidar for profiling atmospheric water vapor, clouds, and aerosols.

    PubMed

    Goldsmith, J E; Blair, F H; Bisson, S E; Turner, D D

    1998-07-20

    We describe an operational, self-contained, fully autonomous Raman lidar system that has been developed for unattended, around-the-clock atmospheric profiling of water vapor, aerosols, and clouds. During a 1996 three-week intensive observational period, the system operated during all periods of good weather (339 out of 504 h), including one continuous five-day period. The system is based on a dual-field-of-view design that provides excellent daytime capability without sacrificing nighttime performance. It is fully computer automated and runs unattended following a simple, brief (~5-min) start-up period. We discuss the theory and design of the system and present detailed analyses of the derivation of water-vapor profiles from the lidar measurements.

  6. Vertical profiles of aerosol and black carbon in the Arctic: a seasonal phenomenology along 2 years (2011-2012) of field campaigns

    NASA Astrophysics Data System (ADS)

    Ferrero, Luca; Cappelletti, David; Busetto, Maurizio; Mazzola, Mauro; Lupi, Angelo; Lanconelli, Christian; Becagli, Silvia; Traversi, Rita; Caiazzo, Laura; Giardi, Fabio; Moroni, Beatrice; Crocchianti, Stefano; Fierz, Martin; Močnik, Griša; Sangiorgi, Giorgia; Perrone, Maria G.; Maturilli, Marion; Vitale, Vito; Udisti, Roberto; Bolzacchini, Ezio

    2016-10-01

    We present results from a systematic study of vertical profiles of aerosol number size distribution and black carbon (BC) concentrations conducted in the Arctic, over Ny-Ålesund (Svalbard). The campaign lasted 2 years (2011-2012) and resulted in 200 vertical profiles measured by means of a tethered balloon (up to 1200 m a.g.l.) during the spring and summer seasons. In addition, chemical analysis of filter samples, aerosol size distribution and a full set of meteorological parameters were determined at ground. The collected experimental data allowed a classification of the vertical profiles into different typologies, which allowed us to describe the seasonal phenomenology of vertical aerosol properties in the Arctic. During spring, four main types of profiles were found and their behavior was related to the main aerosol and atmospheric dynamics occurring at the measuring site. Background conditions generated homogenous profiles. Transport events caused an increase of aerosol concentration with altitude. High Arctic haze pollution trapped below thermal inversions promoted a decrease of aerosol concentration with altitude. Finally, ground-based plumes of locally formed secondary aerosol determined profiles with decreasing aerosol concentration located at different altitude as a function of size. During the summer season, the impact from shipping caused aerosol and BC pollution plumes to be constrained close to the ground, indicating that increasing shipping emissions in the Arctic could bring anthropogenic aerosol and BC in the Arctic summer, affecting the climate.

  7. Global Aerosol Distributions Derived From the CALIPSO Observations

    NASA Astrophysics Data System (ADS)

    Kittaka, C.; Winker, D.; Omar, A.; Liu, Z.; Vaughan, M.; Trepte, C.

    2008-12-01

    Since June 2006, CALIPSO continues to provide routine and systematic measurements of lidar backscatter at two wavelengths, 532 and 1064 nm. As an active sensor, the quality of the measurement is nearly insensitive to surface properties allowing quantitative measurements in regions that are problematic to passive sensors. In particular, aerosol and cloud observations in the polar regions and desert areas are possible with the CALIPSO lidar through the different seasons of a year. The CALIPSO level 2 products, which include aerosol and cloud vertical profiles along tracks, reveal, for the first time, the multi-layer structure of aerosols and clouds on a global scale. This allows not only a depiction of aerosols in relation to clouds, but also the investigation of the interaction between aerosols and clouds. In this study, we present global distributions of aerosol in terms of season, layer height, aerosol species, and in relation to clouds using two years of CALIPSO observations. The CALIPSO aerosol extinction data sets under clear sky are evaluated against the AERONET aerosol optical depth (AOD) and the MODIS AOD collection 5 data sets. The agreement and discrepancies from these comparisons are characterized regionally and investigated using other CALIPSO observable and retrieved parameters. Furthermore, aerosols above clouds and in the vicinity of clouds are examined on a global scale. The implications for aerosol radiative forcing are discussed, highlighting the new and interesting aerosol features obtained from CALIPSO observations.

  8. Aerosol Products from The Future Space Lidar AEOLUS

    NASA Astrophysics Data System (ADS)

    Martinet, Pauline; Dabas, Alain; Lever, Vincent; Flamant, Pierre; Huber, Dorit

    2016-06-01

    Ready for launch by the end of 2016, the Doppler lidar mission AEOLUS from the European Space Agency (ESA) will be the first High-Spectral Resolution Lidar (HSRL) in space. Operating in the UV, it implements two detection channels for aerosol and molecular backscatter. The system is primarily designed for the measurement of winds, but the HSRL capability enables the measurement of the particulate backscatter and extinction coefficients without any a priori assumption on the aerosol type. The level-2A (L2A) processor has been developed for these measurements and tested with synthetic data. The results show good aerosol backscatter profiles can be retrieved. Extinction coefficients are reasonable but do not reach the quality of backscatter coefficients. A precise, full, radiometric calibration of the lidar is required. A major limitation of the system is a single polarization component of the light is detected leading to an underestimation of backscatter coefficients when the atmospheric particles are depolarizing. The vertical resolution goes from 250 meters in the lowest part of the atmosphere, to 2 km in the lower stratosphere. The maximum altitude can reach above 20km. The basic horizontal averaging is 90km. Averaging on shorter distances (down to a few km) are possible but require a sufficient signal to noise ratio.

  9. Influence of the vertical absorption profile of mixed Asian dust plumes on aerosol direct radiative forcing over East Asia

    NASA Astrophysics Data System (ADS)

    Noh, Young Min; Lee, Kwonho; Kim, Kwanchul; Shin, Sung-Kyun; Müller, Detlef; Shin, Dong Ho

    2016-08-01

    We estimate the aerosol direct radiative forcing (ADRF) and heating rate profiles of mixed East Asian dust plumes in the solar wavelength region ranging from 0.25 to 4.0 μm using the Santa Barbara Discrete Ordinate Atmospheric Radiative Transfer (SBDART) code. Vertical profiles of aerosol extinction coefficients and single-scattering albedos (SSA) were derived from measurements with a multi-wavelength Raman lidar system. The data are used as input parameters for our radiative transfer calculations. We considered four cases of radiative forcing in SBDART: 1. dust, 2. pollution, 3. mixed dust plume and the use of vertical profiles of SSA, and 4. mixed dust plumes and the use of column-averaged values of SSA. In our sensitivity study we examined the influence of SSA and aerosol layer height on our results. The ADRF at the surface and in the atmosphere shows a small dependence on the specific shape of the aerosol extinction vertical profile and its light-absorption property for all four cases. In contrast, at the top of the atmosphere (TOA), the ADRF is largely affected by the vertical distribution of the aerosols extinction. This effect increases if the light-absorption capacity (decrease of SSA) of the aerosols increases. We find different radiative effects in situations in which two layers of aerosols had different light-absorption properties. The largest difference was observed at the TOA for an absorbing aerosol layer at high altitude in which we considered in one case the vertical profile of SSA and in another case the column-averaged SSA only. The ADRF at the TOA increases when the light-absorbing aerosol layer is located above 3 km altitude. The differences between height-resolved SSA, which can be obtained from lidar data, and total layer-mean SSA indicates that the use of a layer-mean SSA can be rather misleading as it can induce a large error in the calculation of the ADRF at the TOA, which in turn may cause errors in the vertical profiles of heating rates.

  10. Wavelength dependent near-range lidar profiling of smog aerosol over Athens

    NASA Astrophysics Data System (ADS)

    Stachlewska, Iwona S.; Marinou, Eleni; Engelmann, Ronny; Costa Surós, Montserrat; Kottas, Mickael; Baars, Holger; Janicka, Lucja; Solomos, Stavros; Heese, Birgit; Kumala, Wojciech; Tsekeri, Alexandra; Binietoglou, Ioannis; Markowicz, Krzysztof M.; Amiridis, Vassilis; Balis, Dimitris; Althausen, Dietrich; Wandinger, Ulla; Ansmann, Albert

    2016-04-01

    Recently, the ACTRIS2 JRA1 field campaign focusing on joint remote and in-situ sensing of absorbing aerosols has been conducted in Athens (http://actris-athens.eu). In the frame of the ACTRIS2 BL-Smog TNA, co-located measurements of the near-range lidar receiver (NARLa) of the University of Warsaw with the multi-wavelength PollyXT lidar of the National Observatory of Athens were performed. The excellent capacities of the PollyXT-NOA lidar, equipped with eight far-range channels (355, 355s, 387, 407, 532, 532s, 607, and 1064nm) and two near-range channels (532 and 607 nm), were enhanced by integrating the NARLa for simultaneous observations. By using the NARLa, equipped with the elastic channels (355 and 532nm) and Raman channels (387 and 607nm), the wavelength dependence of the aerosol particles properties within boundary layer was captured. The dominant conditions observed during the JRA1 period were the fresh winter smog layers occurring in lowermost boundary layer over Athens. NARLa provided profiles as close to surface as 50m, thus the data obtained in the near-range were used for the incomplete overlap region of the far-field channels. With NARLa we assessed the overlap at 355 and 532nm wavelengths and concluded on the possibility of using the single near-range 532 nm channel for the overlap correction in both VIS and UV channels of the PollyXT-NOA. As a result, the obtained lidar profiles are expected to be more consistent with the sunphotometer measurements. In the future, the GARRLiC code can be applied on the synergy of combined near and far range lidar profiles with AERONET data sets in order to study improvement on the inversion results.

  11. Light Scattering by Aerosols Over the Remote Ocean: Clear-Sky Point and Column Radiative Closure Studies

    NASA Astrophysics Data System (ADS)

    Fridlind, A. M.; Jacobson, M. Z.

    2001-12-01

    Field data gathered by ship and aircraft during leg 2 of the First Aerosol Characterization Experiment (ACE 1) were used to study clear-sky radiative closure over the remote Southern Ocean. Closure was evaluated by comparing observations with modeled values of: (i) aerosol light scattering coefficients in the marine boundary layer and free troposphere, (ii) total aerosol optical depth, and (iii) total solar radiation at the ocean surface. Point modeling using the ship data benefited from an existing study of closure on the ship, expanding the number of data points considered in that study from 22 to 887. Point and column modeling using the aircraft data provide the first such studies to date. Aerosol light scattering coefficients were calculated from size-distributed measurements of aerosol chemical composition and number concentration, and were compared with observations at three wavelengths (450, 550, and 700 nm) on both ship and aircraft. Point closure on the ship could be achieved at all wavelengths for both total and hemispheric backscattering coefficients if the model accounted for experimental uncertainties in aerosol chemistry, nephelometer nonidealities, and the likely nonsphericity of dried sea salt aerosols. Point closure on the aircraft could be achieved at most wavelengths for total scattering coefficients, but could not be achieved at any wavelengths for hemispheric backscattering coefficients. Deviations between predicted and observed backscattering coefficients on the aircraft were widely scattered rather than biased, indicating that a low signal to noise ratio in observed backscattering coefficients was the likely cause for lack of closure. Aerosol optical depth and solar radiation at the ocean surface were calculated for the two days with clear-sky periods when the aircraft measured aerosol profiles near the ship. Input gas and meteorological data were the observed profiles of ozone, water vapor, temperature, and pressure from the surface to

  12. TOMS Validation Based on Profiles of Aerosol Properties in the Lower Troposphere as Obtained with Light Aircraft Systems

    NASA Technical Reports Server (NTRS)

    Prospero, Joseph M.; Maring, Hal; Savoie, Dennis

    2003-01-01

    The goal of the University of Miami Aerosol Group (UMAG) in this project was to make measurements of vertical profiles of aerosol properties and aerosol optical depth using a light aircraft. The UMAG developed a light aircraft aerosol package (LAAP) that was used in light aircraft (Cessna 172) during the Puerto Rico Dust Experiment (PRIDE). This field campaign took place on Puerto Rico during July 2000. Design details and results from the use of the LAAP were presented at TOMS Science team meetings on April 1998, April 1999, and May 2000. Results from the LAAP collected during the PRIDE Experiment were presented at the Fall Meeting of the American Geophysical Union, December 2000. Some of the results from the LAAP collected during the PRIDE Experiment have been accepted for publication in the Journal of Geophysical Research in a "topical section" made up of papers from the PRIDE Program.

  13. Aerosol Optical Properties Measured Onboard the Ronald H. Brown During ACE Asia as a Function of Aerosol Chemical Composition and Source Region

    NASA Technical Reports Server (NTRS)

    Quinn, P. K.; Coffman, D. J.; Bates, T. S.; Welton, E. J.; Covert, D. S.; Miller, T. L.; Johnson, J. E.; Maria, S.; Russell, L.; Arimoto, R.

    2004-01-01

    During the ACE Asia intensive field campaign conducted in the spring of 2001 aerosol properties were measured onboard the R/V Ronald H. Brown to study the effects of the Asian aerosol on atmospheric chemistry and climate in downwind regions. Aerosol properties measured in the marine boundary layer included chemical composition; number size distribution; and light scattering, hemispheric backscattering, and absorption coefficients. In addition, optical depth and vertical profiles of aerosol 180 deg backscatter were measured. Aerosol within the ACE Asia study region was found to be a complex mixture resulting from marine, pollution, volcanic, and dust sources. Presented here as a function of air mass source region are the mass fractions of the dominant aerosol chemical components, the fraction of the scattering measured at the surface due to each component, mass scattering efficiencies of the individual components, aerosol scattering and absorption coefficients, single scattering albedo, Angstrom exponents, optical depth, and vertical profiles of aerosol extinction. All results except aerosol optical depth and the vertical profiles of aerosol extinction are reported at a relative humidity of 55 +/- 5%. An over-determined data set was collected so that measured and calculated aerosol properties could be compared, internal consistency in the data set could be assessed, and sources of uncertainty could be identified. By taking into account non-sphericity of the dust aerosol, calculated and measured aerosol mass and scattering coefficients agreed within overall experimental uncertainties. Differences between measured and calculated aerosol absorption coefficients were not within reasonable uncertainty limits, however, and may indicate the inability of Mie theory and the assumption of internally mixed homogeneous spheres to predict absorption by the ACE Asia aerosol. Mass scattering efficiencies of non-sea salt sulfate aerosol, sea salt, submicron particulate organic

  14. Vertical profiling of aerosol hygroscopic properties in the planetary boundary layer during the PEGASOS campaigns

    NASA Astrophysics Data System (ADS)

    Rosati, B.; Gysel, M.; Rubach, F.; Mentel, T. F.; Goger, B.; Poulain, L.; Schlag, P.; Miettinen, P.; Pajunoja, A.; Virtanen, A.; Bialek, J.; Klein Baltink, H.; Henzing, J. S.; Größ, J.; Gobbi, G. P.; Wiedensohler, A.; Kiendler-Scharr, A.; O'Dowd, C.; Decesari, S.; Facchini, M. C.; Weingartner, E.; Baltensperger, U.

    2015-03-01

    Airborne measurements of the aerosol hygroscopic and optical properties as well as chemical composition were performed in the Netherlands and northern Italy on board of a Zeppelin NT airship during the PEGASOS field campaigns in 2012. The vertical changes in aerosol properties during the development of the mixing layer were studied. Hygroscopic growth factors (GF) at 95% relative humidity were determined using the white-light humidified optical particles spectrometer (WHOPS) for dry diameters of 300 and 500 nm particles. These measurements were supplemented by an aerosol mass spectrometer (AMS) and an aethalometer providing information on the aerosol chemical composition. Several vertical profiles between 100 and 700 m a.g. were flown just after sunrise close to the San Pietro Capofiume ground station in the Po Valley, Italy. During the early morning hours the lowest layer (newly developing mixing layer) contained a high nitrate fraction (20%) which was coupled with enhanced hygroscopic growth. In the layer above (residual layer) small nitrate fractions of ~ 2% were measured as well as low GFs. After full mixing of the layers, typically around noon and with increased temperature, the nitrate fraction decreased to 2% at all altitudes and led to similar hygroscopicity values as found in the residual layer. These distinct vertical and temporal changes underline the importance of airborne campaigns to study aerosol properties during the development of the mixed layer. The aerosol was externally mixed with 22 and 67% of the 500 nm particles in the range GF < 1.1 and GF > 1.5, respectively. Contributors to the non-hygroscopic mode in the observed size range are most likely mineral dust and biological material. Mean hygroscopicity parameters (κ) were 0.34, 0.19 and 0.18 for particles in the newly forming mixing layer, residual layer and fully mixed layer, respectively. These results agree well with those from chemical analysis which found values of κ = 0.27, 0.21 and 0

  15. Measurement of tropospheric aerosol in São Paulo area using a new upgraded Raman LIDAR system

    NASA Astrophysics Data System (ADS)

    Landulfo, Eduardo; Rodrigues, Patrícia F.; da Silva Lopes, Fábio Juliano; Bourayou, Riad

    2012-11-01

    Elastic backscatter LIDAR systems have been used to determine aerosol profile concentration in several areas such as weather, pollution and air quality monitoring. In order to determine the aerosol extinction and backscattering profiles, the Klett inversion method is largely used, but this method suffers from lack of information since there are two unknown variables to be determined using only one measured LIDAR signal, and assumption of the LIDAR ratio (the relation between the extinction and backscattering coefficients) is needed. When a Raman LIDAR system is used, the inelastic backscattering signal is affected by aerosol extinction but not by aerosol backscatter, which allows this LIDAR to uniquely determine extinction and backscattering coefficients without any assumptions or any collocated instruments. The MSP-LIDAR system, set-up in a highly dense suburban area in the city of São Paulo, has been upgraded to a Raman LIDAR, and in its actual 6-channel configuration allows it to monitor elastic backscatter at 355 and 532 nm together with nitrogen and water vapor Raman backscatters at 387nm and 608 nm and 408nm and 660 nm, respectively. Thus, the measurements of aerosol backscattering, extinction coefficients and water vapor mixing ratio in the Planetary Boundary Layer (PBL) are becoming available. The system will provide the important meteorological parameters such as Aerosol Optical Depth (AOD) and will be used for the study of aerosol variations in lower troposphere over the city of São Paulo, air quality monitoring and for estimation of humidity impact on the aerosol optical properties, without any a priori assumption. This study will present the first results obtained with this upgraded LIDAR system, demonstrating the high quality of obtained aerosol and water vapor data. For that purpose, we compared the data obtained with the new MSP-Raman LIDAR with a mobile Raman LIDAR collocated at the Center for Lasers and Applications, Nuclear and Energy Research

  16. Inter-comparison of CALIPSO and CloudSat retrieved profiles of aerosol and cloud microphysical parameters with aircraft profiles over a tropical region

    NASA Astrophysics Data System (ADS)

    Padmakumari, B.; Harikishan, G.; Maheskumar, R. S.

    2016-05-01

    Satellites play a major role in understanding the spatial and vertical distribution of aerosols and cloud microphysical parameters over a large area. However, the inherent limitations in satellite retrievals can be improved through inter-comparisons with airborne platforms. Over the Indian sub-continent, the vertical profiles retrieved from space-borne lidar such as CALIOP (Cloud-Aerosol LIdar with Orthogonal Polarization) on board the satellite CALIPSO and Cloud Profiling Radar (CPR) on board the satellite CloudSat were inter- compared with the aircraft observations conducted during Cloud Aerosol Interactions and Precipitation Enhancement Experiment (CAIPEEX). In the absence of high clouds, both aircraft and CALIOP showed similar features of aerosol layering and water-ice cloud signatures. As CALIOP could not penetrate the thick clouds, the aerosol information below the cloud is missed. While the aircraft could measure high concentrations below the cloud base and above the low clouds in the presence of high clouds. The aircraft derived liquid water content (LWC) and droplet effective radii (Re) showed steady increase from cloud base to cloud top with a variable cloud droplet number concentration (CDNC). While the CloudSat derived LWC, CDNC and Re showed increase from the cloud top to cloud base in contradiction to the aircraft measurements. The CloudSat profiles are underestimated as compared to the corresponding aircraft profiles. Validation of satellite retrieved vertical profiles with aircraft measurements is very much essential over the tropics to improve the retrieval algorithms and to constrain the uncertainties in the regional cloud parameterization schemes.

  17. Marli: Mars Lidar for Global Wind Profiles and Aerosol Profiles from Orbit

    NASA Technical Reports Server (NTRS)

    Abshire, J. B.; Guzewich, S. D.; Smith, M. D.; Riris, H.; Sun, X.; Gentry, B. M.; Yu, A.; Allan, G. R.

    2016-01-01

    The Mars Exploration Analysis Group's Next Orbiter Science Analysis Group (NEXSAG) has recently identified atmospheric wind measurements as one of 5 top compelling science objectives for a future Mars orbiter. To date, only isolated lander observations of martian winds exist. Winds are the key variable to understand atmospheric transport and answer fundamental questions about the three primary cycles of the martian climate: CO2, H2O, and dust. However, the direct lack of observations and imprecise and indirect inferences from temperature observations leave many basic questions about the atmospheric circulation unanswered. In addition to addressing high priority science questions, direct wind observations from orbit would help validate 3D general circulation models (GCMs) while also providing key input to atmospheric reanalyses. The dust and CO2 cycles on Mars are partially coupled and their influences on the atmospheric circulation modify the global wind field. Dust absorbs solar infrared radiation and its variable spatial distribution forces changes in the atmospheric temperature and wind fields. Thus it is important to simultaneously measure the height-resolved wind and dust profiles. MARLI provides a unique capability to observe these variables continuously, day and night, from orbit.

  18. [Research on source profile of aerosol organic compounds in leather plant].

    PubMed

    Wang, Bo-Guang; Zhou, Yan; Feng, Zhi-Cheng; Liu, Hui-Xuan

    2009-04-15

    Through investigating current air pollution condition for PM10 in every factories of different style leather plants in Pearl River Delta, characteristic profile of semi-volatile organic compounds in PM10 emitted from leather factories and their contents were researched by using ultrasonic and gas chromatography and mass spectrum technology. The 6 types of organic compounds containing 46 species in total were found in the collected samples, including phenyl compounds, alcohols, PAHs, acids, esters and amides. The concentrations of PM10 in leather tanning plant, leather dying plant and man-made leather plant were 678.5, 454.5, 498.6 microgm x m(-3) respectively, and concentration of organic compounds in PM10 were 10.04, 6.89, 14.21 microg x m(-3) in sequence. The more important type of pollutants in each leather plants had higher contribution to total organic mass as follows, esters and amides in tanning plants profile account for 43.47% and 36.51% respectively; esters and alcohols in dying plants profiles account for 52.52% and 16.16% respectively; esters and amide in man-made leather plant have the highest content and account for 57.07% and 24.17% respectively. In the aerosol organic source profiles of tested leather plants, 9-octadecenamide was the abundant important species with the weight of 26.15% in tanning plant, and Bis(2-ethylhexyl) phthalate was up to 44.19% in the dying plant, and Bis(2-ethylhexyl) maleate and 1-hydroxy-piperidine had obviously higher weight in man-made plant than the other two plants.

  19. Analyses of scattering characteristics of chosen anthropogenic aerosols

    NASA Astrophysics Data System (ADS)

    Kaszczuk, Miroslawa; Mierczyk, Zygmunt; Muzal, Michal

    2008-10-01

    In the work, analyses of scattering profile of chosen anthropogenic aerosols for two wavelengths (λ1 = 1064 nm and λ2 = 532 nm) were made. As an example of anthropogenic aerosol three different pyrotechnic mixtures (DM11, M2, M16) were taken. Main parameters of smoke particles were firstly analyzed and well described, taking particle shape and size into special consideration. Shape of particles was analyzed on the basis of SEM pictures, and particle size was measured. Participation of particles in each fixed fraction characterized by range of sizes was analyzed and parameters of smoke particles of characteristic sizes and function describing aerosol size distribution (ASD) were determinated. Analyses of scattering profiles were carried out on the basis of both model of scattering on spherical and nonspherical particles. In the case of spherical particles Rayleigh-Mie model was used and for nonspherical particles analyses firstly model of spheroids was used, and then Rayleigh-Mie one. For each characteristic particle one calculated value of four parameters (effective scattering cross section σSCA, effective backscattering cross section σBSCA, scattering efficiency QSCA, backscattering efficiency QBSCA) and value of backscattering coefficient β for whole particles population. Obtained results were compared with the same parameters calculated for natural aerosol (cirrus cloud).

  20. The E-PROFILE network of automatic LIDARS and ceilometers for operational monitoring of cloud base, aerosols and volcanic ash

    NASA Astrophysics Data System (ADS)

    Haefele, Alexander; Martucci, Giovanni; Haffelin, Martial; Besson, Florence; Lehmann, Volker

    2014-05-01

    During the last years it has been shown that ceilometers are cost effective instruments for vertical profiling of aerosols with proven skills for volcanic plumes detection. As a reaction to the eruptions of the Icelandic volcanoes in 2010 and 2011 and upon recommendation of the COST ES0702 action EG-CLIMET, EUMETNET created the E-PROFILE activity as part of the observation programme which is supported by 18 national meteorological services. E-PROFILE is the continuation of the operational RADAR wind-profiler network E-WINPROF. The new objective of E-PROFILE is to integrate the approximately 700 ceilometers of the E-PROFILE country members into a European network providing vertical profiles for the monitoring of cloud base, aerosols and volcanic ash. A standardized calibration procedure is being developed in collaboration with the COST Action ES1303 TOPROF to provide profile information homogeneously across the network. The information will be distributed in real time and visualized on an interactive map. We present a detailed description of the activity and report on the current status of the development.

  1. Comparison of Aerosol Classification From Airborne High Spectral Resolution Lidar and the CALIPSO Vertical Feature Mask

    NASA Technical Reports Server (NTRS)

    Burton, Sharon P.; Ferrare, Rich A.; Omar, Ali H.; Vaughan, Mark A.; Rogers, Raymond R.; Hostetler, Chris a.; Hair, Johnathan W.; Obland, Michael D.; Butler, Carolyn F.; Cook, Anthony L.; Harper, David B.

    2012-01-01

    Knowledge of aerosol composition and vertical distribution is crucial for assessing the impact of aerosols on climate. In addition, aerosol classification is a key input to CALIOP aerosol retrievals, since CALIOP requires an inference of the lidar ratio in order to estimate the effects of aerosol extinction and backscattering. In contrast, the NASA airborne HSRL-1 directly measures both aerosol extinction and backscatter, and therefore the lidar ratio (extinction-to-backscatter ratio). Four aerosol intensive properties from HSRL-1 are combined to infer aerosol type. Aerosol classification results from HSRL-1 are used here to validate the CALIOP aerosol type inferences.

  2. Aerosol and Cloud Interaction Observed From High Spectral Resolution Lidar Data

    NASA Technical Reports Server (NTRS)

    Su, Wenying; Schuster, Gregory L.; Loeb, Norman G.; Rogers, Raymond R.; Ferrare, Richard A.; Hostetler, Chris A.; Hair, Johnathan W.; Obland, Michael D.

    2008-01-01

    Recent studies utilizing satellite retrievals have shown a strong correlation between aerosol optical depth (AOD) and cloud cover. However, these retrievals from passive sensors are subject to many limitations, including cloud adjacency (or 3D) effects, possible cloud contamination, uncertainty in the AOD retrieval. Some of these limitations do not exist in High Spectral Resolution Lidar (HSRL) observations; for instance, HSRL observations are not a ected by cloud adjacency effects, are less prone to cloud contamination, and offer accurate aerosol property measurements (backscatter coefficient, extinction coefficient, lidar ratio, backscatter Angstrom exponent,and aerosol optical depth) at a neospatial resolution (less than 100 m) in the vicinity of clouds. Hence, the HSRL provides an important dataset for studying aerosol and cloud interaction. In this study, we statistically analyze aircraft-based HSRL profiles according to their distance from the nearest cloud, assuring that all profile comparisons are subject to the same large-scale meteorological conditions. Our results indicate that AODs from HSRL are about 17% higher in the proximity of clouds (approximately 100 m) than far away from clouds (4.5 km), which is much smaller than the reported cloud 3D effect on AOD retrievals. The backscatter and extinction coefficients also systematically increase in the vicinity of clouds, which can be explained by aerosol swelling in the high relative humidity (RH) environment and/or aerosol growth through in cloud processing (albeit not conclusively). On the other hand, we do not observe a systematic trend in lidar ratio; we hypothesize that this is caused by the opposite effects of aerosol swelling and aerosol in-cloud processing on the lidar ratio. Finally, the observed backscatter Angstrom exponent (BAE) does not show a consistent trend because of the complicated relationship between BAE and RH. We demonstrate that BAE should not be used as a surrogate for Angstrom

  3. Long-range transport of aerosols from agriculture crop residue burning in Indo-Gangetic Plains—A study using LIDAR, ground measurements and satellite data

    NASA Astrophysics Data System (ADS)

    Badarinath, K. V. S.; Kumar Kharol, Shailesh; Rani Sharma, Anu

    2009-01-01

    Agriculture crop residue burning in tropics is an important source of atmospheric aerosols and monitoring their long-range transport is an important element in climate change studies. Synchronous measurements using micro-pulsed lidar, MICROTOPS-II sun photometer, multi-filter rotating shadow band radiometer (MFRSR) on aerosol optical depth and ground reaching solar irradiance were carried at an urban location in central region of India. Aerosol backscatter profiles obtained from micro-pulse lidar showed elevated aerosol layers up to ~3 km on certain days during October 2007. Satellite data observations on aerosol properties suggested transport of particles from agriculture crop residue burning in Indo-Gangetic Plains over large regions. Radiative forcing of aerosols estimated from SBDART model with input information on aerosol chemical properties, aerosol optical depth and single scattering albedo and broadband solar irradiance measurements using MFRSR showed good correlation (R=0.98).

  4. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    NASA Astrophysics Data System (ADS)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2016-01-01

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of aerosol optical depths (AODs) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in northern India. The WRF-Chem model is found to heavily underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model's low bias is due to aerosol extinctions below ˜ 2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day-1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently

  5. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    NASA Astrophysics Data System (ADS)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-01

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day-1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently

  6. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    DOE PAGES

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2016-01-18

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of aerosol optical depths (AODs) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in northern India. The WRF-Chem model is found to heavily underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model's low bias is due to aerosol extinctions below  ∼  2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profiles averaged over Southmore » Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to −0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and

  7. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    SciTech Connect

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2016-01-01

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of aerosol optical depths (AODs) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in northern India. The WRF-Chem model is found to heavily underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model's low bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to

  8. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    SciTech Connect

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-19

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond

  9. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    DOE PAGES

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-19

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AODmore » and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond

  10. Results of a comprehensive atmospheric aerosol-radiation experiment in the southwestern United States. I - Size distribution, extinction optical depth and vertical profiles of aerosols suspended in the atmosphere. II - Radiation flux measurements and

    NASA Technical Reports Server (NTRS)

    Deluisi, J. J.; Furukawa, F. M.; Gillette, D. A.; Schuster, B. G.; Charlson, R. J.; Porch, W. M.; Fegley, R. W.; Herman, B. M.; Rabinoff, R. A.; Twitty, J. T.

    1976-01-01

    Results are reported for a field test that was aimed at acquiring a sufficient set of measurements of aerosol properties required as input for radiative-transfer calculations relevant to the earth's radiation balance. These measurements include aerosol extinction and size distributions, vertical profiles of aerosols, and radiation fluxes. Physically consistent, vertically inhomogeneous models of the aerosol characteristics of a turbid atmosphere over a desert and an agricultural region are constructed by using direct and indirect sampling techniques. These results are applied for a theoretical interpretation of airborne radiation-flux measurements. The absorption term of the complex refractive index of aerosols is estimated, a regional variation in the refractive index is noted, and the magnitude of solar-radiation absorption by aerosols and atmospheric molecules is determined.

  11. Sensitivity Analysis on Fu-Liou-Gu Radiative Transfer Model for different lidar aerosol and cloud profiles

    NASA Astrophysics Data System (ADS)

    Lolli, Simone; Madonna, Fabio; Rosoldi, Marco; Pappalardo, Gelsomina; Welton, Ellsworth J.

    2016-04-01

    The aerosol and cloud impact on climate change is evaluated in terms of enhancement or reduction of the radiative energy, or heat, available in the atmosphere and at the Earth's surface, from the surface (SFC) to the Top Of the Atmosphere (TOA) covering a spectral range from the UV (extraterrestrial shortwave solar radiation) to the far-IR (outgoing terrestrial longwave radiation). Systematic Lidar network measurements from permanent observational sites across the globe are available from the beginning of this current millennium. From the retrieved lidar atmospheric extinction profiles, inputted in the Fu-Liou-Gu (FLG) Radiative Transfer code, it is possible to evaluate the net radiative effect and heating rate of the different aerosol species and clouds. Nevertheless, the lidar instruments may use different techniques (elastic lidar, Raman lidar, multi-wavelength lidar, etc) that translate into uncertainty of the lidar extinction retrieval. The goal of this study is to assess, applying a MonteCarlo technique and the FLG Radiative Transfer model, the sensitivity in calculating the net radiative effect and heating rate of aerosols and clouds for the different lidar techniques, using both synthetic and real lidar data. This sensitivity study is the first step to implement an automatic algorithm to retrieve the net radiative forcing effect of aerosols and clouds from the long records of aerosol measurements available in the frame of EARLINET and MPLNET lidar networks.

  12. Oxygen depth profiling by resonant backscattering and glow discharge optical emission spectroscopy of Ti-6Al-4V alloy oxidized by ion implantation and plasma based treatment

    NASA Astrophysics Data System (ADS)

    Nsengiyumva, S.; Topic, M.; Pichon, L.; Comrie, C. M.; Mtshali, C.

    2016-10-01

    Oxygen depth profiling by means of 16O(α,α)16O backscattering and glow discharge optical emission spectroscopy (GDOES) was investigated in two different sets of Ti-6Al-4V samples. The first set was made of Ti-6Al-4V samples implanted at room temperature and 550 °C with 50 and 150 keV O+ ions at fluences ranging from 1.5 × 1017 to 6.0 × 1017 ions/cm2. The second set consisted of Ti-6Al-4V samples treated at 550 °C for 7 h and 24 h under low pressure (8 Pa) oxygen, eventually with RF plasma activation. These results are part of a wider investigation on Ti-6Al-4V motivated by recent publications which have shown that an oxide layer can enhance hydrogen absorption and can then promote Ti-6Al-4V alloys as efficient hydrogen storage materials. The results obtained by the two characterization techniques were compared and discussed, enabling to adjust the dependence to the oxygen concentration of the sputtering rates to be used in the time-to-depth transformation required in GDOES analysis. Considering the low thickness of oxidized alloy, usual procedures employed in GDOES depth calculation were indeed not adapted. Once calibrated thanks to the resonant RBS, GDOES can then be easily employed as fast characterization of oxidized and/or hydrogenated surface of Ti-6Al-4V. The obtained results show that the oxygen content into the surface oxidized layer slightly increases in samples implanted at higher fluence and higher temperature. However the overall oxidized layer thickness (<200 nm) remains within the projected ion depth range and is not significantly increased by thermal diffusion at 550 °C. Taken into account the initial oxide layer, the incorporated oxygen quantity mainly corresponds to the implanted fluence but it can be slightly higher with 550 °C implantation, indicating a slight additional oxidation by residual oxygen or surface contamination. The oxygen penetrations and contents in samples oxidized by thermally activated diffusion treatments were more

  13. An Accuracy Assessment of the CALIOP/CALIPSO Version 2/Version 3 Daytime Aerosol Extinction Product Based on a Detailed Multi-Sensor, Multi-Platform Case Study

    NASA Technical Reports Server (NTRS)

    Kacenelenbogen, M.; Vaughan, M. A.; Redemann, J.; Hoff, R. M.; Rogers, R. R.; Ferrare, R. A.; Russell, P. B.; Hostetler, C. A.; Hair, J. W.; Holben, B. N.

    2011-01-01

    The Cloud Aerosol LIdar with Orthogonal Polarization (CALIOP), on board the CALIPSO platform, has measured profiles of total attenuated backscatter coefficient (level 1 products) since June 2006. CALIOP s level 2 products, such as the aerosol backscatter and extinction coefficient profiles, are retrieved using a complex succession of automated algorithms. The goal of this study is to help identify potential shortcomings in the CALIOP version 2 level 2 aerosol extinction product and to illustrate some of the motivation for the changes that have been introduced in the next version of CALIOP data (version 3, released in June 2010). To help illustrate the potential factors contributing to the uncertainty of the CALIOP aerosol extinction retrieval, we focus on a one-day, multi-instrument, multiplatform comparison study during the CALIPSO and Twilight Zone (CATZ) validation campaign on 4 August 2007. On that day, we observe a consistency in the Aerosol Optical Depth (AOD) values recorded by four different instruments (i.e. spaceborne MODerate Imaging Spectroradiometer, MODIS: 0.67 and POLarization and Directionality of Earth s Reflectances, POLDER: 0.58, airborne High Spectral Resolution Lidar, HSRL: 0.52 and ground-based AErosol RObotic NETwork, AERONET: 0.48 to 0.73) while CALIOP AOD is a factor of two lower (0.32 at 532 nm). This case study illustrates the following potential sources of uncertainty in the CALIOP AOD: (i) CALIOP s low signal-to-noise ratio (SNR) leading to the misclassification and/or lack of aerosol layer identification, especially close to the Earth s surface; (ii) the cloud contamination of CALIOP version 2 aerosol backscatter and extinction profiles; (iii) potentially erroneous assumptions of the aerosol extinction-to-backscatter ratio (Sa) used in CALIOP s extinction retrievals; and (iv) calibration coefficient biases in the CALIOP daytime attenuated backscatter coefficient profiles. The use of version 3 CALIOP extinction retrieval for our case

  14. Aerosol Profile Measurements from the NASA Langley Research Center Airborne High Spectral Resolution Lidar

    NASA Technical Reports Server (NTRS)

    Obland, Michael D.; Hostetler, Chris A.; Ferrare, Richard A.; Hair, John W.; Roers, Raymond R.; Burton, Sharon P.; Cook, Anthony L.; Harper, David B.

    2008-01-01

    Since achieving first light in December of 2005, the NASA Langley Research Center (LaRC) Airborne High Spectral Resolution Lidar (HSRL) has been involved in seven field campaigns, accumulating over 450 hours of science data across more than 120 flights. Data from the instrument have been used in a variety of studies including validation and comparison with the Cloud- Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite mission, aerosol property retrievals combining passive and active instrument measurements, aerosol type identification, aerosol-cloud interactions, and cloud top and planetary boundary layer (PBL) height determinations. Measurements and lessons learned from the HSRL are leading towards next-generation HSRL instrument designs that will enable even further studies of aerosol intensive and extensive parameters and the effects of aerosols on the climate system. This paper will highlight several of the areas in which the NASA Airborne HSRL is making contributions to climate science.

  15. The effects of increasing atmospheric ozone on biogenic monoterpene profiles and the formation of secondary aerosols

    NASA Astrophysics Data System (ADS)

    Pinto, Delia M.; Tiiva, Päivi; Miettinen, Pasi; Joutsensaari, Jorma; Kokkola, Harri; Nerg, Anne-Marja; Laaksonen, Ari; Holopainen, Jarmo K.

    Monoterpenes are biogenic volatile organic compounds (BVOCs) which play an important role in plant adaptation to stresses, atmospheric chemistry, plant-plant and plant-insect interactions. In this study, we determined whether ozonolysis can influence the monoterpenes in the headspace of cabbage. The monoterpenes were mixed with an air-flow enriched with 100, 200 or 400 ppbv of ozone (O 3) in a Teflon chamber. The changes in the monoterpene and O 3 concentrations, and the formation of secondary organic aerosols (SOA) were determined during ozonolysis. Furthermore, the monoterpene reactions with O 3 and OH were modelled using reaction kinetics equations. The results showed that all of the monoterpenes were unequally affected: α-thujene, sabinene and D-limonene were affected to the greatest extend, whereas the 1,8-cineole concentration did not change. In addition, plant monoterpene emissions reduced the O 3 concentration by 12-24%. The SOA formation was dependent on O 3 concentration. At 100 ppbv of O 3, virtually no new particles were formed but clear SOA formation was observed at the higher ozone concentrations. The modelled results showed rather good agreements for α-pinene and 1,8-cineole, whereas the measured concentrations were clearly lower compared to modelled values for sabinene and limonene. In summary, O 3-quenching by monoterpenes occurs beyond the boundary layer of leaves and results in a decreased O 3 concentration, altered monoterpene profiles and SOA formation.

  16. Cloud and Aerosol Properties, Precipitable Water, and Profiles of Temperature and Water Vapor from MODIS

    NASA Technical Reports Server (NTRS)

    King, Michael D.; Menzel, W. Paul; Kaufman, Yoram J.; Tanre, Didier; Gao, Bo-Cai; Platnick, Steven; Ackerman, Steven A.; Remer, Lorraine A.; Pincus, Robert; Hubanks, Paul A.

    2003-01-01

    The Moderate Resolution Imaging Spectroradiometer (MODIS) is an earth-viewing sensor that flies on the Earth Observing System (EOS) Terra and Aqua satellites, launched in 1999 and 2002, respectively. MODIS scans a swath width of 2330 km that is sufficiently wide to provide nearly complete global coverage every two days from a polar-orbiting, sun-synchronous, platform at an altitude of 705 km. MODIS provides images in 36 spectral bands between 0.415 and 14.235 pm with spatial resolutions of 250 m (2 bands), 500 m (5 bands) and 1000 m (29 bands). These bands have been carefully selected to en- able advanced studies of land, ocean, and atmospheric properties. Twenty-six bands are used to derive atmospheric properties such as cloud mask, atmospheric profiles, aerosol properties, total precipitable water, and cloud properties. In this paper we describe each of these atmospheric data products, including characteristics of each of these products such as file size, spatial resolution used in producing the product, and data availability.

  17. SAM II aerosol profile measurements, Poker Flat, Alaska; July 16-19, 1979

    NASA Technical Reports Server (NTRS)

    Mccormick, M. P.; Chu, W. P.; Mcmaster, L. R.; Grams, G. W.; Herman, B. M.; Pepin, T. J.; Russell, P. B.; Swissler, T. J.

    1981-01-01

    SAM II satellite measurements during the July 1979 Poker Flat mission, yielded an aerosol extinction coefficient of 0.0004/km at 1.0 micron wavelength, in the region of the stratospheric aerosol mixing ratio peak (12-16 km). The stratospheric aerosol optical depth for these data, calculated from the tropopause through 30 km, is approximately 0.001. These results are consistent with the average 1979 summertime values found throughout the Arctic.

  18. CALIPSO-inferred aerosol direct radiative effects: Bias estimates using ground-based Raman lidars

    NASA Astrophysics Data System (ADS)

    Thorsen, Tyler J.; Fu, Qiang

    2015-12-01

    Observational constraints on the change in the radiative energy budget caused by the presence of aerosols, i.e., the aerosol direct radiative effect (DRE), have recently been made using observations from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite (CALIPSO). CALIPSO observations have the potential to provide improved global estimates of aerosol DRE compared to passive sensor-derived estimates due to CALIPSO's ability to perform vertically resolved aerosol retrievals over all surface types and over cloud. In this study, uncertainties in CALIPSO-inferred aerosol DRE are estimated using multiple years of observations from the Atmospheric Radiation Measurement (ARM) program's Raman lidars at midlatitude and tropical sites. We find that CALIPSO is unable to detect all radiatively significant aerosol, resulting in an underestimate in the magnitude of the aerosol DRE by 30-50% at the two ARM sites. The undetected aerosol is likely the consequence of random noise in CALIPSO measurements and therefore will affect global observations as well. This suggests that the global aerosol DRE inferred from CALIPSO observations are likely too weak. Also examined is the impact of the ratio of extinction-to-backscatter (i.e., the lidar ratio) whose value CALIPSO retrievals must assume to obtain the aerosol extinction profile. It is shown that if CALIPSO can reproduce the climatological value of the lidar ratio at a given location, then the aerosol DRE there can be accurately calculated (within about 3%).

  19. LASE measurements of water vapor and aerosol profiles during the Plains Elevated Convection at Night (PECAN) field experiment

    NASA Astrophysics Data System (ADS)

    Nehrir, A. R.; Ferrare, R. A.; Kooi, S. A.; Butler, C. F.; Notari, A.; Hair, J. W.; Collins, J. E., Jr.; Ismail, S.

    2015-12-01

    The Lidar Atmospheric Sensing Experiment (LASE) system was deployed on the NASA DC-8 aircraft during the Plains Elevated Convection At Night (PECAN) field experiment, which was conducted during June-July 2015 over the central and southern plains. LASE is an active remote sensor that employs the differential absorption lidar (DIAL) technique to measure range resolved profiles of water vapor and aerosols above and below the aircraft. The DC-8 conducted nine local science flights from June 30- July 14 where LASE sampled water vapor and aerosol fields in support of the PECAN primary science objectives relating to better understanding nocturnal Mesoscale Convective Systems (MCSs), Convective Initiation (CI), the Low Level Jet (LLJ), bores, and to compare different airborne and ground based measurements. LASE observed large spatial and temporal variability in water vapor and aerosol distributions in advance of nocturnal MCSs, across bores resulting from MCS outflow boundaries, and across the LLJ associated with the development of MCSs and CI. An overview of the LASE data collected during the PECAN field experiment will be presented where emphasis will be placed on variability of water vapor profiles in the vicinity of severe storms and intense convection in the central and southern plains. Preliminary comparisons show good agreement between coincident LASE and radiosonde water vapor profiles. In addition, an advanced water vapor DIAL system being developed at NASA Langley will be discussed.

  20. The Potential of The Synergy of Sunphotometer and Lidar Data to Validate Vertical Profiles of The Aerosol Mass Concentration Estimated by An Air Quality Model

    NASA Astrophysics Data System (ADS)

    Siomos, N.; Filioglou, M.; Poupkou, A.; Liora, N.; Dimopoulos, S.; Melas, D.; Chaikovsky, A.; Balis, D. S.

    2016-06-01

    Vertical profiles of the aerosol mass concentration derived by the Lidar/Radiometer Inversion Code (LIRIC), that uses combined sunphotometer and lidar data, were used in order to validate the aerosol mass concentration profiles estimated by the air quality model CAMx. Lidar and CIMEL measurements performed at the Laboratory of Atmospheric Physics of the Aristotle University of Thessaloniki, Greece (40.5N, 22.9E) from the period 2013-2014 were used in this study.

  1. Retrievals of Extensive and Intensive Aerosol Parameters from Vertical Profiles of Extinction Coefficient Acquired by the MAESTRO Occultation Spectrometer: Case Study of Sarychev Volcano Plumes

    NASA Astrophysics Data System (ADS)

    Saha, A.; O'Neill, N. T.; McElroy, C. T.; Sioris, C.; Zou, J.

    2011-12-01

    The Canadian MAESTRO (Measurement of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation) instrument aboard the SCISAT-1 Satellite is an aerosol profiling occultation device that is part of the ACE (Atmospheric Chemistry Experiment) mission. This spectrometer produces spectra of aerosol extinction profiles above the upper troposphere. The extinction coefficient spectra permit the discrimination of sub-micron (fine mode) and super-micron (coarse mode) contributions and, in principle, the retrieval of fine mode effective radius. Retrievals applied to lower stratospheric and upper tropospheric aerosol plumes resulting from the eruption of the Sarychev-peak volcano in June of 2009 are presented. Preliminary results indicate that the fine and coarse mode discrimination and the particle sizing capability are coherent with available information on Sarychev aerosols.

  2. Vertical profiles of atmospheric fluorescent aerosols observed by a mutil-channel lidar spectrometer system

    NASA Astrophysics Data System (ADS)

    Huang, Z.; Huang, J.; Zhou, T.; Sugimoto, N.; Bi, J.

    2015-12-01

    Zhongwei Huang1*, Jianping Huang1, Tian Zhou1, Nobuo Sugimoto2, Jianrong Bi1 and Jinsen Shi11Key Laboratory for Semi-Arid Climate Change of the Ministry of Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou, China. 2Atmospheric Environment Division, National Institutes for Environmental Studies, Tsukuba, Japan Email: huangzhongwei@lzu.edu.cn Abstract Atmospheric aerosols have a significant impact on regional and globe climate. The challenge in quantifying aerosol direct radiative forcing and aerosol-cloud interactions arises from large spatial and temporal heterogeneity of aerosol concentrations, compositions, sizes, shape and optical properties (IPCC, 2007). Lidar offers some remarkable advantages for determining the vertical structure of atmospheric aerosols and their related optical properties. To investigate the characterization of atmospheric aerosols (especially bioaerosols) with high spatial and temporal resolution, we developed a Raman/fluorescence/polarization lidar system employed a multi-channel spectrometer, with capabilities of providing measurements of Raman scattering and laser-induced fluorescence excitation at 355 nm from atmospheric aerosols. Meanwhile, the lidar system operated polarization measurements both at 355nm and 532nm wavelengths, aiming to obtain more information of aerosols. It employs a high power pulsed laser and a received telescope with 350mm diameter. The receiver could simultaneously detect a wide fluorescent spectrum about 178 nm with spectral resolution 5.7 nm, mainly including an F/3.7 Crossed Czerny-Turner spectrograph, a grating (1200 gr/mm) and a PMT array with 32 photocathode elements. Vertical structure of fluorescent aerosols in the atmosphere was observed by the developed lidar system at four sites across northwest China, during 2014 spring field observation that conducted by Lanzhou University. It has been proved that the developed lidar could detect the fluorescent aerosols with high temporal and

  3. New capabilities for space-based cloud and aerosols measurements: The Cloud-Aerosol Transport System (CATS)

    NASA Astrophysics Data System (ADS)

    Yorks, J. E.; McGill, M. J.; Hlavka, D. L.; Palm, S. P.; Hart, W. D.; Nowottnick, E. P.; Vaughan, M.; Rodier, S. D.; Colarco, P. R.; da Silva, A.; Buchard-Marchant, V.

    2013-12-01

    Current uncertainties in cloud and aerosol properties limit our ability to accurately model the Earth's climate system and predict climate change. These limitations are due primarily to difficulties in adequately measuring aerosols and clouds on a global scale. NASA's A-Train satellites provide an unprecedented opportunity to address these uncertainties. In particular, the Cloud-Aerosol Lidar Infrared Pathfinder Spaceborne Observations (CALIPSO) satellite provides vertical profiles of cloud and aerosol properties. The CALIOP lidar onboard CALIPSO has reached its seventh year of operation, well past its expected lifetime. The ATLID lidar on EarthCARE is not expected to launch until 2016 or later. If the CALIOP lidar fails before a new mission is operational, there will be a gap in global lidar measurements. The Cloud-Aerosol Transport System (CATS), built at NASA Goddard Space Flight Center as a payload for the International Space Station (ISS), is set to launch in the summer of 2014. CATS is an elastic backscatter lidar with three wavelengths (1064, 532, 355 nm) and HSRL capability at 532 nm. Depolarization measurements will be made at all three wavelengths. The ISS orbit is a 51 degree inclination orbit at an altitude of about 405 km. This orbit provides more comprehensive coverage of the tropics and mid-latitudes than sun-synchronous orbiting sensors, with nearly a three day repeat cycle. Thus, science applications of CATS include cloud and aerosol climate studies, air quality monitoring, and smoke/volcanic plume tracking. The primary science objectives of CATS include: continuing the CALIPSO aerosol and cloud vertical profile data record, providing near real time data to support operational applications such as air quality modeling, and advancing technology in support of future mission development using the HSRL channel. Furthermore, the vertical profiles of cloud and aerosol properties provided by CATS will complement current and future passive satellite

  4. Compact airborne Raman lidar for profiling aerosol, water vapor and clouds.

    PubMed

    Liu, Bo; Wang, Zhien; Cai, Yong; Wechsler, Perry; Kuestner, William; Burkhart, Matthew; Welch, Wayne

    2014-08-25

    A compact airborne Raman lidar system, which can perform water vapor and aerosol measurements both during nighttime and daytime is described. The system design, setup and the data processing methods are described in the paper. The Raman lidar was tested on University of Wyoming King Air research aircraft (UWKA) during the Wyoming King Air PBL Exploratory Experiment (KAPEE) in 2010. An observation showing clouds, aerosols and a dry line is presented to illustrate the lidar detection capabilities. Comparisons of the water vapor and aerosol measurements using the Raman lidar and other in situ airborne instruments show good agreement. PMID:25321266

  5. Compact airborne Raman lidar for profiling aerosol, water vapor and clouds.

    PubMed

    Liu, Bo; Wang, Zhien; Cai, Yong; Wechsler, Perry; Kuestner, William; Burkhart, Matthew; Welch, Wayne

    2014-08-25

    A compact airborne Raman lidar system, which can perform water vapor and aerosol measurements both during nighttime and daytime is described. The system design, setup and the data processing methods are described in the paper. The Raman lidar was tested on University of Wyoming King Air research aircraft (UWKA) during the Wyoming King Air PBL Exploratory Experiment (KAPEE) in 2010. An observation showing clouds, aerosols and a dry line is presented to illustrate the lidar detection capabilities. Comparisons of the water vapor and aerosol measurements using the Raman lidar and other in situ airborne instruments show good agreement.

  6. On observing acoustic backscattering from salinity turbulence.

    PubMed

    Goodman, Louis; Sastre-Cordova, Marcos M

    2011-08-01

    It has been hypothesized that at sufficiently high levels of oceanic salinity turbulence it should be possible to observe acoustic backscattering. However, there have been limited in situ measurements to confirm this hypothesis. Using an autonomous underwater vehicle equipped with upward and downward looking 1.2 MHz acoustic Doppler current profilers and with turbulence and fine scale sensors, measurements were performed in a region of intense turbulence and a strong salinity gradient. The approach taken was to correlate variations in the backscattered acoustic intensity, I, with a theoretical acoustic backscattering cross section per volume for salinity turbulence, σ(s), to obtain an estimated scattering cross section per volume, σ(e). Results indicated that of order 50% of the observed region was characterized by salinity turbulence induced backscattering. PMID:21877785

  7. On observing acoustic backscattering from salinity turbulence.

    PubMed

    Goodman, Louis; Sastre-Cordova, Marcos M

    2011-08-01

    It has been hypothesized that at sufficiently high levels of oceanic salinity turbulence it should be possible to observe acoustic backscattering. However, there have been limited in situ measurements to confirm this hypothesis. Using an autonomous underwater vehicle equipped with upward and downward looking 1.2 MHz acoustic Doppler current profilers and with turbulence and fine scale sensors, measurements were performed in a region of intense turbulence and a strong salinity gradient. The approach taken was to correlate variations in the backscattered acoustic intensity, I, with a theoretical acoustic backscattering cross section per volume for salinity turbulence, σ(s), to obtain an estimated scattering cross section per volume, σ(e). Results indicated that of order 50% of the observed region was characterized by salinity turbulence induced backscattering.

  8. CALIPSO-inferred aerosol direct radiative effects: Bias estimates using ground-based Raman lidars

    NASA Astrophysics Data System (ADS)

    Thorsen, T. J.; Fu, Q.

    2015-12-01

    Observational constraints on the change in radiative energy budget caused by the presence of aerosols, i.e. the aerosol direct radiative effect (DRE), have recently been made using observations from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite (CALIPSO). CALIPSO observations have the potential to provide improved global estimates of aerosol DRE compared to passive sensor-derived estimates due to CALIPSO's ability to perform vertically-resolved aerosol retrievals over all surface types and over cloud. In this study we estimate the uncertainties in CALIPSO-inferred aerosol DRE using multiple years of observations from the Atmospheric Radiation Measurement (ARM) program's Raman lidars (RL) at midlatitude and tropical sites. Examined are assumptions about the ratio of extinction-to-backscatter (i.e. the lidar ratio) made by the CALIPSO retrievals, which are needed to retrieve the aerosol extinction profile. The lidar ratio is shown to introduce minimal error in the mean aerosol DRE at the top-of-atmosphere and surface. It is also shown that CALIPSO is unable to detection all radiatively-significant aerosol, resulting in an underestimate in the magnitude of the aerosol DRE. Therefore, global estimates of the aerosol DRE inferred from CALIPSO are likely too weak.

  9. Seasonal variations in Titan's stratosphere observed with Cassini/CIRS: temperature, trace molecular gas and aerosol mixing ratio profiles

    NASA Astrophysics Data System (ADS)

    Vinatier, S.; Bézard, B.; Anderson, C.; Teanby, N.; Lebonnois, S.; Rannou, P.; de Kok, R.; T. CIRS Team

    2013-09-01

    Titan's northern spring equinox occurred in August 2009. General Circulation Models (e.g. [1]) predict strong modifications of the global circulation in this period, with formation of two circulation cells instead of the pole-to-pole cell that occurred during northern winter. This winter single cell, which had its descending branch at the north pole, was at the origin of the enrichment of molecular abundances and high stratopause temperatures observed by Cassini/CIRS at high northern latitudes (e.g., [2], [3], [4], [5]). The predicted dynamical seasonal variations after the equinox have strong impact on the spatial distributions of trace gas, temperature and aerosol abundances. We will present here an analysis of CIRS limbgeometry datasets acquired in 2010, 2011 and 2012 that we used to monitor the seasonal evolution of the vertical profiles of temperature, molecular (C2H2, C2H6, HCN, ...) and aerosol abundances.

  10. Comparison of stratospheric aerosol and gas experiment I (SAGE I) and Umkehr ozone profiles including a search for Umkehr aerosol effects

    SciTech Connect

    Newchurch, M.J.

    1986-01-01

    After briefly reviewing ozone depletion predictions from atmospheric models and results from trend analysis of Umkehr data, this paper outlines the Umkehr method for deducing the vertical profile of ozone and reviews the theoretical and empirical studies of the aerosol effect on Umkehr measurements. A brief description of the Stratospheric Aerosol and Gas Experiment I (SAGE I) is followed by a method for approximating the best representation of the conditions over the Umkehr ground site as seen by the SAGE I satellite. Using a spatially weighted average of SAGE I events derived from an autocorrelation analysis, the authors find 337 co-located SAGE I and Umkehr events. The approximate total column ozone measured by SAGE I is 5% higher than that measured by Umkehr on average. Most of this difference resides in Umkehr layer two, three, and four, while layers seven, eight, and nine contain small differences in average ozone content. Intercomparison with four other ozone studies indicates agreement between SAGE I and SBUV in most layers and at most Umkehr stations north of 30/sup 0/. However, significant differences in Umkehr layer eight between SAGE I and SBUV remain. Ozone differences between SAGE I and Umkehr are strong functions of both total column ozone and season in the lower layers but not in the upper layers.

  11. Airborne lidar measurements of El Chichon stratospheric aerosols, October 1982 to November 1982

    NASA Technical Reports Server (NTRS)

    Mccormick, M. P.; Osborn, M. T.

    1985-01-01

    A coordinated flight mission to determine the spatial distribution and aerosol characteristics of the El Chichon produced stratospheric aerosol was flown in October to November 1982. The mission covered 46 deg N to 46 deg S and included rendezvous between balloon-, airplane-, and satellite-borne sensors. The lidar data from the flight mission are presented. Representative profiles of lidar backscatter ratio, plots of the integrated backscattering function versus latitude, and contours of backscatter mixing ratio versus altitude and latitude are given. In addition, tables containing numerical values of the backscatter ratio and backscattering functions versus altitude are supplied for each profile. The bulk of the material produced by the El Chichon eruptions of late March 10 to early April 1982 resided between latitudes from 5 to 7 deg S to 35 to 37 deg N and was concentrated above 21 km in a layer that peaked at 23 to 25 km. In this latitude region, peak scattering ratios at a wavelength of 0.6943 micron were approximately 24. The results of this mission are presented in a ready-to-use format for atmospheric and climatic studies.

  12. Dynamic coherent backscattering mirror

    PubMed Central

    Xu, M.

    2016-01-01

    The phase of multiply scattered light has recently attracted considerable interest. Coherent backscattering is a striking phenomenon of multiple scattered light in which the coherence of light survives multiple scattering in a random medium and is observable in the direction space as an enhancement of the intensity of backscattered light within a cone around the retroreflection direction. Reciprocity also leads to enhancement of backscattering light in the spatial space. The random medium behaves as a reciprocity mirror which robustly converts a diverging incident beam into a converging backscattering one focusing at a conjugate spot in space. Here we first analyze theoretically this coherent backscattering mirror (CBM) phenomenon and then demonstrate the capability of CBM compensating and correcting both static and dynamic phase distortions occurring along the optical path. CBM may offer novel approaches for high speed dynamic phase corrections in optical systems and find applications in sensing and navigation. PMID:26937296

  13. Aerosol characteristics in the UTLS region: A satellite-based study over north India

    NASA Astrophysics Data System (ADS)

    Srivastava, A. K.; Misra, A.; Kanawade, Vijay P.; Devara, P. C. S.

    2016-01-01

    Vertical profiles of aerosol backscatter coefficient and depolarization ratio, obtained from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite, were studied in the upper troposphere and lower stratosphere (UTLS) region over North India (21-30° N and 72-90° E), covering the highly polluted Indo-Gangetic Plain (IGP) for one-year period from December 2011 to November 2012. An enhanced aerosol layer was observed between 15 and 18 km altitude, in the vicinity of tropopause, with a broad layer depth of about 2 km. The aerosol layer showed strong seasonal, monthly as well as day and night time variability, with a peak value of backscatter coefficient during monsoon season (˜5.54 × 10-3 sr-1 in September). The corresponding depolarization ratio indicates anisotropic (non-spherical) nature of particles. The aerosol layer was found to be highly linked with the variability in tropopause height, showing a positive correlation between tropopause height and the height of maximum backscatter coefficient (correlation coefficient of 0.8). However, it was found to be negatively correlated with the integrated backscatter coefficient (IBC), with a correlation coefficient of 0.3. We further analyzed outgoing long-wave radiation (OLR) data during the study period to investigate the link between the observed enhanced aerosol layer in the UTLS region and prevailing deep convective activities over the study region. Low values of OLR during monsoon (about 214 W m-2) indicate the occurrence of deep convection over this region, which may cause a large-scale circulation-driven vertical transport of boundary-layer pollution into the atmosphere of UTLS region. Results may have potential implications for better understanding and assessing the chemical and radiative impacts of these aerosols in the tropical UTLS region.

  14. Aerosol analysis techniques and results from micro pulse lidar

    NASA Technical Reports Server (NTRS)

    Hlavka, Dennis L.; Spinhirne, James D.; Campbell, James R.; Reagan, John A.; Powell, Donna

    1998-01-01

    The effect of clouds and aerosol on the atmospheric energy balance is a key global change problem. Full knowledge of aerosol distributions is difficult to obtain by passive sensing alone. Aerosol and cloud retrievals in several important areas can be significantly improved with active remote sensing by lidar. Micro Pulse Lidar (MPL) is an aerosol and cloud profilometer that provides a detailed picture of the vertical structure of boundary layer and elevated dust or smoke plume aerosols. MPL is a compact, fully eyesafe, ground-based, zenith pointing instrument capable of full-time, long-term unattended operation at 523 nm. In October of 1993, MPL began taking full-time measurements for the Atmospheric Radiation Measurement (ARM) program at its Southern Great Plains (SGP) site and has since expanded to ARM sites in the Tropical West Pacific (TWP) and the North Slope of Alaska (NSA). Other MPL's are moving out to some of the 60 world-wide Aerosol Robotic Network (AERONET) sites which are already equipped with automatic sun-sky scanning spectral radiometers providing total column optical depth measurements. Twelve additional MPL's have been purchased by NASA to add to the aerosol and cloud database of the EOS ground validation network. The original MPL vertical resolution was 300 meters but the newer versions have a vertical resolution of 30 meters. These expanding data sets offer a significant new resource for atmospheric radiation analysis. Under the direction of Jim Spinhirne, the MPL analysis team at NASA/GSFC has developed instrument correction and backscatter analysis techniques for ARM to detect cloud boundaries and analyze vertical aerosol structures. A summary of MPL applications is found in Hlavka (1997). With the aid of independent total column optical depth instruments such as the Multifilter Rotating Shadowband Radiometer (MFRSR) at the ARM sites or sun photometers at the AERONET sites, the MPL data can be calibrated, and time-resolved vertical profiles of

  15. Vertical resolved separation of aerosol types using CALIPSO level-2 product

    NASA Astrophysics Data System (ADS)

    Giannakaki, Elina; Balis, Dimitris; Amiridis, Vassilis

    2011-11-01

    A lidar-based method was used to separate profiles of optical parameters due to different aerosol types over different European Aerosol Research LIdar NETwork (EARLINET) stations. The method makes uses of particle backscatter profiles at 532 nm and vertically resolved linear particle depolarization ratio measurements at the same wavelength. Values of particle depolarization ratio of 'pure' aerosol types (Saharan dust, biomass burning aerosols, anthropogenic aerosols, Volcanic ash aerosols) were taken from literature. Cases of CALIPSO space-borne lidar system were selected on the basis of different mixing state of the atmosphere over EARLINET stations. To identify the origin of air-masses four-day air mass back trajectories were computed using HYbrid Single-Particle Langrangian Integrated Trajectory (HYSPLIT) model, for different arrival heights, for the location and time under study was used. Also, the Dust REgional Atmospheric Modeling (DREAM) model was used to identify cases where dust from Saharan region was affecting the place under study. For our analysis we have used Atmospheric Volume Description (AVD), Cloud-Aerosol Discrimination (CAD) and extinction Quality Control (QC) flags to screen out CALIOP data. The method was applied for different horizontal resolution of 5, 25, 45 and 105 km. The height-resolved lidar results were finally compared with column-integrated products obtained with Aerosol Robotic Network Sun photometer (AERONET) in order to see to what extent Sun photometer columnar data are representative when different aerosol layers are present in the atmosphere.

  16. Scanning tropospheric ozone and aerosol lidar with double-gated photomultipliers.

    PubMed

    Machol, Janet L; Marchbanks, Richard D; Senff, Christoph J; McCarty, Brandi J; Eberhard, Wynn L; Brewer, William A; Richter, Ronald A; Alvarez, Raul J; Law, Daniel C; Weickmann, Ann M; Sandberg, Scott P

    2009-01-20

    The Ozone Profiling Atmospheric Lidar is a scanning four-wavelength ultraviolet differential absorption lidar that measures tropospheric ozone and aerosols. Derived profiles from the lidar data include ozone concentration, aerosol extinction, and calibrated aerosol backscatter. Aerosol calibrations assume a clear air region aloft. Other products include cloud base heights, aerosol layer heights, and scans of particulate plumes from aircraft. The aerosol data range from 280 m to 12 km with 5 m range resolution, while the ozone data ranges from 280 m to about 1.2 km with 100 m resolution. In horizontally homogeneous atmospheres, data from multiple-elevation angles is combined to reduce the minimum altitude of the aerosol and ozone profiles to about 20 m. The lidar design, the characterization of the photomultiplier tubes, ozone and aerosol analysis techniques, and sample data are described. Also discussed is a double-gating technique to shorten the gated turn-on time of the photomultiplier tubes, and thereby reduce the detection of background light and the outgoing laser pulse.

  17. Scanning tropospheric ozone and aerosol lidar with double-gated photomultipliers.

    PubMed

    Machol, Janet L; Marchbanks, Richard D; Senff, Christoph J; McCarty, Brandi J; Eberhard, Wynn L; Brewer, William A; Richter, Ronald A; Alvarez, Raul J; Law, Daniel C; Weickmann, Ann M; Sandberg, Scott P

    2009-01-20

    The Ozone Profiling Atmospheric Lidar is a scanning four-wavelength ultraviolet differential absorption lidar that measures tropospheric ozone and aerosols. Derived profiles from the lidar data include ozone concentration, aerosol extinction, and calibrated aerosol backscatter. Aerosol calibrations assume a clear air region aloft. Other products include cloud base heights, aerosol layer heights, and scans of particulate plumes from aircraft. The aerosol data range from 280 m to 12 km with 5 m range resolution, while the ozone data ranges from 280 m to about 1.2 km with 100 m resolution. In horizontally homogeneous atmospheres, data from multiple-elevation angles is combined to reduce the minimum altitude of the aerosol and ozone profiles to about 20 m. The lidar design, the characterization of the photomultiplier tubes, ozone and aerosol analysis techniques, and sample data are described. Also discussed is a double-gating technique to shorten the gated turn-on time of the photomultiplier tubes, and thereby reduce the detection of background light and the outgoing laser pulse. PMID:19151820

  18. Study of aerosol hygroscopic events over the Cabauw experimental site for atmospheric research (CESAR) using the multi-wavelength Raman lidar Caeli

    NASA Astrophysics Data System (ADS)

    Fernández, A. J.; Apituley, A.; Veselovskii, I.; Suvorina, A.; Henzing, J.; Pujadas, M.; Artíñano, B.

    2015-11-01

    This article presents a study of aerosol optical and microphysical properties under different relative humidity (RH) but well mixed layer conditions using optical and microphysical aerosol properties from multi-wavelength (MW) Raman lidar and in-situ aerosol observations collected at the Cabauw Experimental Site for Atmospheric Research (CESAR). Two hygroscopic events are described through 3 backscatter (β) and 2 extinction (α) coefficients which in turn provide intensive parameters such as the backscatter-related Ångström exponent (åβ) and the lidar ratio (LR). Along with it, profiles of RH were inferred from Raman lidar observations and therefore, as a result of varying humidity conditions, a shift on the aerosol optical properties can be described. Thus, it is observed that as RH increases, aerosols uptake water vapour, augment their size and consequently the åβ diminishes whereas the LR increases. The enhancement factor based on the backscatter coefficient at 532 nm, which characterizes the aerosol from hygroscopic standpoint, is also estimated. Finally, microphysical properties that are necessary for aerosol radiative forcing estimates - such as volume, effective radii, refractive index and size distribution, all vertically resolved - are retrieved using the inversion with regularization. Using this method, two hygroscopic events are described in detail.

  19. Characterizing the Vertical Distribution of Aerosols Over the ARM SGP Site

    SciTech Connect

    Richard Ferrare, Connor Flynn, David Turner

    2009-05-05

    . Analysis of the aerosol and water vapor data collected by the Raman lidar during the 2003 Aerosol IOP indicated that the sensitivity of the lidar was significantly lower than when the lidar was initially deployed. A detailed analysis after the IOP of the long-term dataset demonstrated that the lidar began degrading in early 2002, and that it lost approximately a factor of 4 in sensitivity between 2002 and 2004. We participated in the development of the remediation plan for the system to restore its initial performance. We conducted this refurbishment and upgrade from May- September 2004. This remediation lead to an increase in the signal-to-noise ratio of 10 and 30 for the Raman lidar's water vapor mixing ratio and aerosol backscatter coefficient data, respectively as compared to the signal strengths when the system was first deployed. The DOE ARM Aerosol Lidar Validation Experiment (ALIVE), which was conducted during September 2005, evaluated the impact of these modifications and upgrades on the SGP Raman lidar measurements of aerosol extinction and optical thickness. The CARL modifications significantly improved the accuracy and temporal resolution of the aerosol measurements. Aerosol extinction profiles measured by the Raman lidar were also used to evaluate aerosol extinction profiles and aerosol optical thickness (AOT) simulated by aerosol models as part of the Aerosol module inter-Comparison in global models (AEROCOM) (http://nansen.ipsl.jussieu.fr/AEROCOM/aerocomhome.html) project. There was a wide range in how the models represent the aerosol extinction profiles over the ARM SGP site, even though the average annual AOT represented by the various models and measured by CARL and the Sun photometer were in general agreement, at least within the standard deviations of the averages. There were considerable differences in the average vertical distributions among the models, even among models that had similar average aerosol optical thickness. Deviations between mean

  20. Surface observations of aerosols and vertical ozone profiling: Influence from the Indo Gangetic Plain, biomass burning and LRT

    NASA Astrophysics Data System (ADS)

    Naja, M. K.; Kotamarthi, V. R.; Singh, N.; Phani, D. V.; Dumka, U. C.; Kumar, R.; Ojha, N.; Bhardhwaj, P.; Lal, S.

    2013-12-01

    South Asia is the home to one of the most populated and polluted region (The Indo-Gangetic Plain, IGP) of the world and variety of anthropogenic and biogenic emission sources are exiting in the same region. Despite of the poor understanding of the physical, chemical, and dynamical processes in the lower atmosphere over this region, there are very limited ground based observations in South Asia. In view of this, an observational facility was setup at ARIES, Nainital (29.4N, 79.5E; 1950 m) in the central Himalayas and at two sites in the IGP region for the surface based trace gases and aerosols observations as well as balloon-borne ozone observations. Further, First Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF1), DOE, was setup at ARIES during a GVAX campaign (June 2011-March 2012) and extensive observations of vertical profiling was also carried out using balloons, doppler Lidar, microwave radiometer, wind profiler and ceilometers. Observations of trace gases and aerosols show a clear enhancement during pre-monsoon and a secondary peak during post-monsoon period. The average scattering Angstrom exponent suggests dominance of relatively larger size particles and single scattering albedo indicates more scattering or less absorbing aerosols in this region. Events of the long-range transport are seen, when concentrations of bigger particle are observed to be higher. Apart from LRT, events of downward transport of ozone rich but drier air-masses are also observed. Extensive in-situ observations of ozone, CO, BC, aerosol absorption, scattering and number-concentration, along with back-air trajectories and MODIS fire-counts have been used to demonstrate evidences of the influence of biomass burning over this region. Aerosol organic enrichment and subsequent evolution to predominantly accumulation mode have been observed. This enrichment and its simultaneous size-growth caused it to get brighter during the biomass burning season. A very clear enhancement (20

  1. Spectral variability of the particulate backscattering ratio

    NASA Astrophysics Data System (ADS)

    Whitmire, A. L.; Boss, E.; Cowles, T. J.; Pegau, W. S.

    2007-05-01

    The spectral dependency of the particulate backscattering ratio is relevant in the fields of ocean color inversion, light field modeling, and inferring particle properties from optical measurements. Aside from theoretical predictions for spherical, homogeneous particles, we have very limited knowledge of the actual in situ spectral variability of the particulate backscattering ratio. This work presents results from five research cruises that were conducted over a three-year period. Water column profiles of physical and optical properties were conducted across diverse aquatic environments that offered a wide range of particle populations. The main objective of this research was to examine the behavior of the spectral particulate backscattering ratio in situ, both in terms of its absolute magnitude and its variability across visible wavelengths, using over nine thousand 1-meter binned data points for each of five wavelengths of the spectral particulate backscattering ratio. Our analysis reveals no spectral dependence of the particulate backscattering ratio within our measurement certainty, and a geometric mean value of 0.013 for this dataset. This is lower than the commonly used value of 0.0183 from Petzold’s integrated volume scattering data. Within the first optical depth of the water column, the mean particulate backscattering ratio was 0.010.

  2. Measuring the stratospheric aerosol size distribution profile following the next big volcanic eruption. What is required?

    NASA Astrophysics Data System (ADS)

    Deshler, T.

    2015-12-01

    Two of the key missing features of fresh and evolving volcanic plumes are the particle size distribution and its partitioning into non-volatile ash and volatile sulfate particles. Such information would allow more refined estimates of the evolution and dispersal of the aerosol, of the impacts of the aerosol on radiation and on stratospheric chemistry, and of the overall amount of sulfur injected into the stratosphere. To provide this information aerosol measurements must be sensitive to particles in the 0.1 - 10 μm radius range, with concentration detection thresholds > 0.001 cm-3, and to the total aerosol population. An added bonus would be a size resolved measurement of the non-volatile fraction of the aerosol. The measurements must span the lower and mid stratosphere up to about 30 km. There are no remote measurements which can provide this information. In situ measurements using aerosol and condensation nuclei counters are required. Aircraft platforms are available for measurements up to 20 km, but beyond that requires balloon platforms. Measurements above 20 km would be required for a large volcanic eruption. There are balloon-borne instruments capable of fulfilling all of the measurement requirements; however such instruments are reasonably large and not expendable. The difficulty is deploying the instruments, obtaining the flight permissions from air traffic control, and recovering the instruments after flight. Such difficulties are compounded in the tropics. This talk will detail some previous experience in this area and suggest ways forward to be ready for the next big eruption.

  3. Optical properties of Southern Hemisphere aerosols: Report of the joint CSIRO/NASA study

    NASA Technical Reports Server (NTRS)

    Gras, John L.; Platt, C. Martin; Huffaker, R. Milton; Jones, William D.; Kavaya, Michael J.; Gras, John L.

    1988-01-01

    This study was made in support of the LAWS and GLOBE programs, which aim to design a suitable Doppler lidar system for measuring global winds from a satellite. Observations were taken from 5 deg S to 45 deg S along and off the E and SE Australian coast, thus obtaining representative samples over a large latitude range. Observations were made between 0 and 6 km altitude of aerosol physical and chemical properties in situ from the CSIRO F-27 aircraft; of lidar backscatter coefficients at 10.6 micron wavelength from the F-27 aircraft; of lidar backscatter profiles at 0.694 microns at Sale, SE Australia; and of lidar backscatter profiles at 0.532 microns at Cowley Beach, NE Australia. Both calculations and observations in the free troposphere gave a backscatter coefficient of 1-2 x 10 to the -11/m/sr at 10.6 microns, although the accuracies of the instruments were marginal at this level. Equivalent figures were 2-8 x 10 to the -9/m/sr (aerosol) and 9 x 10 to the -9 to 2 x 10 to the -8/m/sr (lidar) at 0.694 microns wavelength at Sale; and 3.7 x 10 to the -9/m/sr (aerosol) and 10 to the -8 to 10 to the -7/m/sr (lidar) at 0.532 microns wavelength at Cowley Beach. The measured backscatter coefficients at 0.694 and 0.532 microns were consistently higher than the values calculated from aerosol size distributions by factors of typically 2 to 10.

  4. Multistatic aerosol-cloud lidar in space: A theoretical perspective

    NASA Astrophysics Data System (ADS)

    Mishchenko, Michael I.; Alexandrov, Mikhail D.; Cairns, Brian; Travis, Larry D.

    2016-11-01

    Accurate aerosol and cloud retrievals from space remain quite challenging and typically involve solving a severely ill-posed inverse scattering problem. In this Perspective, we formulate in general terms an aerosol and aerosol-cloud interaction space mission concept intended to provide detailed horizontal and vertical profiles of aerosol physical characteristics as well as identify mutually induced changes in the properties of aerosols and clouds. We argue that a natural and feasible way of addressing the ill-posedness of the inverse scattering problem while having an exquisite vertical-profiling capability is to fly a multistatic (including bistatic) lidar system. We analyze theoretically the capabilities of a formation-flying constellation of a primary satellite equipped with a conventional monostatic (backscattering) lidar and one or more additional platforms each hosting a receiver of the scattered laser light. If successfully implemented, this concept would combine the measurement capabilities of a passive multi-angle multi-spectral polarimeter with the vertical profiling capability of a lidar; address the ill-posedness of the inverse problem caused by the highly limited information content of monostatic lidar measurements; address the ill-posedness of the inverse problem caused by vertical integration and surface reflection in passive photopolarimetric measurements; help relax polarization accuracy requirements; eliminate the need for exquisite radiative-transfer modeling of the atmosphere-surface system in data analyses; yield the day-and-night observation capability; provide direct characterization of ground-level aerosols as atmospheric pollutants; and yield direct measurements of polarized bidirectional surface reflectance. We demonstrate, in particular, that supplementing the conventional backscattering lidar with just one additional receiver flown in formation at a scattering angle close to 170° can dramatically increase the information content of the

  5. Airborne High Spectral Resolution Lidar Aerosol Measurements during MILAGRO and TEXAQS/GOMACCS

    NASA Technical Reports Server (NTRS)

    Ferrare, Richard; Hostetler, Chris; Hair, John; Cook Anthony; Harper, David; Burton, Sharon; Clayton, Marian; Clarke, Antony; Russell, Phil; Redemann, Jens

    2007-01-01

    Two1 field experiments conducted during 2006 provided opportunities to investigate the variability of aerosol properties near cities and the impacts of these aerosols on air quality and radiative transfer. The Megacity Initiative: Local and Global Research Observations (MILAGRO) /Megacity Aerosol Experiment in Mexico City (MAX-MEX)/Intercontinental Chemical Transport Experiment-B (INTEX-B) joint experiment conducted during March 2006 investigated the evolution and transport of pollution from Mexico City. The Texas Air Quality Study (TEXAQS)/Gulf of Mexico Atmospheric Composition and Climate Study (GoMACCS) (http://www.al.noaa.gov/2006/) conducted during August and September 2006 investigated climate and air quality in the Houston/Gulf of Mexico region. During both missions, the new NASA Langley airborne High Spectral Resolution Lidar (HSRL) was deployed on the NASA Langley B200 King Air aircraft and measured profiles of aerosol extinction, backscattering, and depolarization to: 1) characterize the spatial and vertical distributions of aerosols, 2) quantify aerosol extinction and optical thickness contributed by various aerosol types, 3) investigate aerosol variability near clouds, 4) evaluate model simulations of aerosol transport, and 5) assess aerosol optical properties derived from a combination of surface, airborne, and satellite measurements.

  6. Raman lidar system for the measurement of water vapor and aerosols in the earth's atmosphere

    NASA Technical Reports Server (NTRS)

    Whiteman, D. N.; Melfi, S. H.; Ferrare, R. A.

    1992-01-01

    A nighttime operating Raman lidar system that is designed for the measurement of high vertical and temporal resolution profiles of the water vapor mixing ratio and the aerosol backscattering ratio is described. The theory of the measurements is presented. Particular attention is given to operational problems that have been solved during the development of the system. Data are presented from Sept. 1987 and described in their meteorological context.

  7. Implementation of Raman lidar for profiling of atmospheric water vapor and aerosols at the SGP CART site

    SciTech Connect

    Goldsmith, J.E.M.; Bisson, S.E.; Blair, F.H.; Whiteman, D.N.; Melfi, S.H.; Ferrare, R.A.

    1994-05-01

    There are clearly identified scientific requirements for continuous profiling of atmospheric water vapor at the SGP CART (southern great plains cloud and radiation testbed) site. Research conducted at several laboratories, including our own collaboration in a previous ARM Instrument Development Project, has demonstrated the suitability of Raman lidar for providing measurements that are an excellent match to those requirements. We are currently building a ruggedized Raman lidar system that will reside permanently at the CART site, and that is computer-automated to minimize requirements for operator interaction. In addition to profiling water vapor through most of the troposphere during nighttime and through the boundary layer during daytime, the lidar will provide quantitative characterizations of aerosols and clouds, including depolarization measurements for particle phase studies.

  8. The Cloud-Aerosol Transport System (CATS): Demonstrating New Techniques for Cloud and Aerosol Measurements

    NASA Astrophysics Data System (ADS)

    Yorks, J. E.; McGill, M. J.; Palm, S. P.; Hlavka, D. L.; Nowottnick, E. P.; Selmer, P. A.

    2015-12-01

    The Cloud-Aerosol Transport System (CATS) is an elastic backscatter lidar that provides vertical profiles of cloud and aerosol properties. The CATS payload has been operating since early February 2015 from the International Space Station (ISS). CATS was designed to operate for six months, and up to three years, providing a combination of operational science, in-space technology demonstration, and technology risk reduction for future Earth Science missions. One of the primary project goals of CATS is to demonstrate technology in support of future space-based lidar mission development. The CATS instrument has been demonstrating the high repetition rate laser and photon counting detection approach to lidar observations, in contrast to the low repetition rate, high energy technique employed by CALIPSO. Due to this technique, cloud and aerosol profile data exhibit high spatial and temporal resolution, which was never before possible from a space-based platform. Another important science goal of the CATS-FO project is accurate determination of aerosol type on a global scale. CATS provided the first space-based depolarization measurements at multiple wavelengths (532 and 1064 nm), and first measurements at 1064 nm from space. The ratio of the depolarization measurements at these two wavelengths enables significant improvement in aerosol typing. The CATS retrievals at 1064 nm also provide improvements to detecting aerosols above clouds. The CATS layer identification algorithm is a threshold-based layer detection method that uses the 1064 nm attenuated scattering ratio and also includes a routine to identify clouds embedded within aerosol layers. This technique allows CATS to detect the full extent of the aerosol layers above the cloud, and differentiate these two layers so that the optical properties can be more accurately determined.

  9. Airborne High Spectral Resolution Lidar Measurements of Aerosol Distributions and Properties during the NASA DISCOVER-AQ Missions

    NASA Astrophysics Data System (ADS)

    Ferrare, R. A.; Hostetler, C. A.; Hair, J. W.; Scarino, A. J.; Burton, S. P.; Harper, D. B.; Cook, A. L.; Berkoff, T.; Rogers, R. R.; Seaman, S. T.; Fenn, M. A.; Sawamura, P.; Clayton, M.; Mueller, D.; Chemyakin, E.; Anderson, B. E.; Beyersdorf, A. J.; Ziemba, L. D.; Crawford, J. H.

    2015-12-01

    The NASA Langley Research Center airborne High Spectral Resolution Lidars, HSRL-1 and HSRL-2, were deployed for the DISCOVER-AQ (Deriving Information on Surface Conditions from COlumn and VERtically Resolved Observations Relevant to Air Quality) missions. DISCOVER-AQ provided systematic and concurrent observations of column-integrated, surface, and vertically-resolved distributions of aerosols and trace gases to improve the interpretation of satellite observations related to air quality. HSRL-1, deployed during the first DISCOVER-AQ mission over the Washington DC-Baltimore region, measured profiles of aerosol backscatter and depolarization (532, 1064 nm) and aerosol extinction and optical thickness (AOT) (532 nm). HSRL-2, the first airborne multiwavelength HSRL, was deployed for the following three DISCOVER-AQ missions over the California Central Valley, Houston, and Denver. HSRL-2 measures profiles of aerosol backscatter and depolarization (355, 532, 1064 nm) and aerosol extinction and AOT (355, 532 nm). Additional HSRL-2 data products include aerosol type, mixed layer depth, and range-resolved aerosol microphysical parameters. The HSRL measurements reveal the temporal, spatial, and vertical variability of aerosol optical properties over these locations. HSRL measurements show that surface PM2.5 concentrations were better correlated with near surface aerosol extinction than AOT scaled by the mixed layer height. During the missions over Washington DC-Baltimore, Houston, and Denver, only about 20-65% of AOT was within the mixed layer. In contrast, nearly all of the AOT was within the mixed layer over the California Central Valley. HSRL-2 retrievals of aerosol fine mode volume concentration and effective radius compare well with coincident airborne in situ measurements and vary with relative humidity. HSRL-2 retrievals of aerosol fine mode volume concentration were also used to derive PM2.5 concentrations which compare well with surface PM2.5 measurements.

  10. Comparison of Aerosol Optical Properties and Water Vapor Among Ground and Airborne Lidars and Sun Photometers During TARFOX

    NASA Technical Reports Server (NTRS)

    Ferrare, R.; Ismail, S.; Browell, E.; Brackett, V.; Clayton, M.; Kooi, S.; Melfi, S. H.; Whiteman, D.; Schwemmer, G.; Evans, K.

    2000-01-01

    We compare aerosol optical thickness (AOT) and precipitable water vapor (PWV) measurements derived from ground and airborne lidars and sun photometers during the Tropospheric Aerosol Radiative Forcing Observational Experiment. Such comparisons are important to verify the consistency between various remote sensing measurements before employing them in any assessment of the impact of aerosols on the global radiation balance. Total scattering ratio and extinction profiles measured by the ground-based NASA Goddard Space Flight Center scanning Raman lidar system, which operated from Wallops Island, Virginia (37.86 deg N, 75.51 deg W); are compared with those measured by the Lidar Atmospheric Sensing Experiment (LASE) airborne lidar system aboard the NASA ER-2 aircraft. Bias and root-mean-square differences indicate that these measurements generally agreed within about 10%. Aerosol extinction profiles and estimates of AOT are derived from both lidar measurements using a value for the aerosol extinction/backscattering ratio S(sub a) = 60 sr for the aerosol extinction/backscattering ratio, which was determined from the Raman lidar measurements. The lidar measurements of AOT are found to be generally within 25% of the AOT measured by the NASA Ames Airborne Tracking Sun Photometer (AATS-6). However, during certain periods the lidar and Sun photometer measurements of AOT differed significantly, possibly because of variations in the aerosol physical characteristics (e.g., size, composition) which affect S(sub a). Estimates of PWV, derived from water vapor mixing ratio profiles measured by LASE, are within 5-10% of PWV derived from the airborne Sun photometer. Aerosol extinction profiles measured by both lidars show that aerosols were generally concentrated in the lowest 2-3 km.

  11. Development the EarthCARE aerosol classification scheme

    NASA Astrophysics Data System (ADS)

    Wandinger, Ulla; Baars, Holger; Hünerbein, Anja; Donovan, Dave; van Zadelhoff, Gerd-Jan; Fischer, Jürgen; von Bismarck, Jonas; Eisinger, Michael; Lajas, Dulce; Wehr, Tobias

    2015-04-01

    The Earth Clouds, Aerosols and Radiation Explorer (EarthCARE) mission is a joint ESA/JAXA mission planned to be launched in 2018. The multi-sensor platform carries a cloud-profiling radar (CPR), a high-spectral-resolution cloud/aerosol lidar (ATLID), a cloud/aerosol multi-spectral imager (MSI), and a three-view broad-band radiometer (BBR). Three out of the four instruments (ATLID, MSI, and BBR) will be able to sense the global aerosol distribution and contribute to the overarching EarthCARE goals of sensor synergy and radiation closure with respect to aerosols. The high-spectral-resolution lidar ATLID obtains profiles of particle extinction and backscatter coefficients, lidar ratio, and linear depolarization ratio as well as the aerosol optical thickness (AOT) at 355 nm. MSI provides AOT at 670 nm (over land and ocean) and 865 nm (over ocean). Next to these primary observables the aerosol type is one of the required products to be derived from both lidar stand-alone and ATLID-MSI synergistic retrievals. ATLID measurements of the aerosol intensive properties (lidar ratio, depolarization ratio) and ATLID-MSI observations of the spectral AOT will provide the basic input for aerosol-type determination. Aerosol typing is needed for the quantification of anthropogenic versus natural aerosol loadings of the atmosphere, the investigation of aerosol-cloud interaction, assimilation purposes, and the validation of atmospheric transport models which carry components like dust, sea salt, smoke and pollution. Furthermore, aerosol classification is a prerequisite for the estimation of direct aerosol radiative forcing and radiative closure studies. With an appropriate underlying microphysical particle description, the categorization of aerosol observations into predefined aerosol types allows us to infer information needed for the calculation of shortwave radiative effects, such as mean particle size, single-scattering albedo, and spectral conversion factors. In order to ensure

  12. Geometrical constraint experimental determination of Raman lidar overlap profile.

    PubMed

    Li, Jian; Li, Chengcai; Zhao, Yiming; Li, Jing; Chu, Yiqi

    2016-06-20

    A simple experimental method to determine the overlap profile of Raman lidar is presented in this paper. Based on Mie and Raman backscattering signals and a geometrically constrained condition, the overlap profile of a Raman lidar system can be determined. Our approach simultaneously retrieves the lidar ratio of aerosols, which is one of the most important sources of uncertainty in the overlap profile determination. The results indicate that the overlap factor is significantly influenced by the lidar ratio in experimental methods. A representative case study indicates that the correction of the overlap profile obtained by this method is practical and feasible.

  13. Geometrical constraint experimental determination of Raman lidar overlap profile.

    PubMed

    Li, Jian; Li, Chengcai; Zhao, Yiming; Li, Jing; Chu, Yiqi

    2016-06-20

    A simple experimental method to determine the overlap profile of Raman lidar is presented in this paper. Based on Mie and Raman backscattering signals and a geometrically constrained condition, the overlap profile of a Raman lidar system can be determined. Our approach simultaneously retrieves the lidar ratio of aerosols, which is one of the most important sources of uncertainty in the overlap profile determination. The results indicate that the overlap factor is significantly influenced by the lidar ratio in experimental methods. A representative case study indicates that the correction of the overlap profile obtained by this method is practical and feasible. PMID:27409119

  14. Shortwave Radiative Fluxes, Solar-Beam Transmissions, and Aerosol Properties: TARFOX and ACE-2 Find More Absorption from Flux Radiometry than from Other Measurements

    NASA Technical Reports Server (NTRS)

    Russell, Philip B.; Redemann, J.; Schmid, B.; Livingston, J. M.; Bergstrom, R. W.; Ramirez, S. A.; Hipskind, R. Stephen (Technical Monitor)

    2001-01-01

    The Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) and the Second Aerosol Characterization Experiment (ACE-2) made simultaneous measurements of shortwave radiative fluxes, solar-beam transmissions, and the aerosols affecting those fluxes and transmissions. Besides the measured fluxes and transmissions, other obtained properties include aerosol scattering and absorption measured in situ at the surface and aloft; aerosol single scattering albedo retrieved from skylight radiances; and aerosol complex refractive index derived by combining profiles of backscatter, extinction, and size distribution. These measurements of North Atlantic boundary layer aerosols impacted by anthropogenic pollution revealed the following characteristic results: (1) Better agreement among different types of remote measurements of aerosols (e.g., optical depth, extinction, and backscattering from sunphotometers, satellites, and lidars) than between remote and in situ measurements; 2) More extinction derived from transmission measurements than from in situ measurements; (3) Larger aerosol absorption inferred from flux radiometry than from other measurements. When the measured relationships between downwelling flux and optical depth (or beam transmission) are used to derive best-fit single scattering albedos for the polluted boundary layer aerosol, both TARFOX and ACE-2 yield midvisible values of 0.90 +/- 0.04. The other techniques give larger single scattering albedos (i.e. less absorption) for the polluted boundary layer, with a typical result of 0.95 +/- 0.04. Although the flux-based results have the virtue of describing the column aerosol unperturbed by sampling, they are subject to questions about representativeness and other uncertainties (e.g., unknown gas absorption). Current uncertainties in aerosol single scattering albedo are large in terms of climate effects. They also have an important influence on aerosol optical depths retrieved from satellite radiances

  15. CART Raman Lidar Aerosol and Water Vapor Measurements in the Vicinity of Clouds

    NASA Technical Reports Server (NTRS)

    Clayton, Marian B.; Ferrare, Richard A.; Turner, David; Newsom, Rob; Sivaraman, Chitra

    2008-01-01

    Aerosol and water vapor profiles acquired by the Raman lidar instrument located at the Climate Research Facility (CRF) at Southern Great Plains (SGP) provide data necessary to investigate the atmospheric variability in the vicinity of clouds near the top of the planetary boundary layer (PBL). Recent CARL upgrades and modifications to the routine processing algorithms afforded the necessarily high temporal and vertical data resolutions for these investigations. CARL measurements are used to investigate the behavior of aerosol backscattering and extinction and their correlation with water vapor and relative humidity.

  16. Potentialities and Limits of ICESAT-2 Observation for Atmospheric Aerosol Investigation

    NASA Astrophysics Data System (ADS)

    Mona, L.; Amodeo, A.; D'Amico, G.

    2016-06-01

    ICESat-2(Ice, Cloud, and land Elevation Satellite-2), slated for launch in 2017, will continue the important observations of ice-sheet elevation change, sea-ice freeboard, and vegetation canopy height begun by ICESat in 2003. Among the other potential applications, ICESat-2 could provide some information about atmospheric aerosol over Polar Regions thanks to the lidar instrument. In this context, it is essential to demonstrate the ICESat-2 capability of providing vertical profiles of the aerosol backscatter coefficient and to define its potentialities and limits. First results of this investigation are reported and will be presented at the conference.

  17. Tropospheric Ozone Lidar Network (TOLNet) - Long-term Tropospheric Ozone and Aerosol Profiling for Satellite Continuity and Process Studies

    NASA Astrophysics Data System (ADS)

    Newchurch, M.; Al-Saadi, J. A.; Alvarez, R. J.; Burris, J.; Cantrell, W.; Chen, G.; De Young, R.; Hardesty, R.; Hoff, R. M.; Kaye, J. A.; kuang, S.; Langford, A. O.; LeBlanc, T.; McDermid, I. S.; McGee, T. J.; Pierce, R.; Senff, C. J.; Sullivan, J. T.; Szykman, J.; Tonnesen, G.; Wang, L.

    2012-12-01

    An interagency research initiative for ground-based ozone and aerosol lidar profiling recently funded by NASA has important applications to air-quality studies in addition to the goal of serving the GEO-CAPE and other air-quality missions. Ozone is a key trace-gas species, a greenhouse gas, and an important pollutant in the troposphere. High spatial and temporal variability of ozone affected by various physical and photochemical processes motivates the high spatio-temporal lidar profiling of tropospheric ozone for improving the simulation and forecasting capability of the photochemical/air-quality models, especially in the boundary layer where the resolution and precision of satellite retrievals are fundamentally limited. It is well known that there are large discrepancies between the surface and upper-air ozone due to titration, surface deposition, diurnal processes, free-tropospheric transport, and other processes. Near-ground ozone profiling has been technically challenging for lidars due to some engineering difficulties, such as near-range saturation, field-of-view overlap, and signal processing issues. This initiative provides an opportunity for us to solve those engineering issues and redesign the lidars aimed at long-term, routine ozone/aerosol observations from the near surface to the top of the troposphere at multiple stations (i.e., NASA/GSFC, NASA/LaRC, NASA/JPL, NOAA/ESRL, UAHuntsville) for addressing the needs of NASA, NOAA, EPA and State/local AQ agencies. We will present the details of the science investigations, current status of the instrumentation development, data access/protocol, and the future goals of this lidar network. Ozone lidar/RAQMS comparison of laminar structures.

  18. The Asian Tropopause Aerosol layer through satellite and balloon-borne measurements combined with modelling approaches.

    NASA Astrophysics Data System (ADS)

    Vernier, J. P.; Fairlie, T. D.; Natarajan, M.; Crawford, J. H.; Baker, N. C.; Wegner, T.; Deshler, T.; Gadhavi, H. S.; Kumar, S.; Singh, A. K.; Jayaraman, A.; Raj, A.; Alladi, H.; Ratnam, M. V.; Pandit, A.; Vignelles, D.; Wienhold, F.; Liu, H.; Kumar, S.

    2015-12-01

    The Asian tropopause Aerosol Layer (ATAL) is a seasonal aerosol feature occurring in the Upper Troposphere and Lower Stratosphere (UTLS) above Asia during the Summer Asian Monsoon. Vertically resolved aerosol backscatter profiles from the Cloud-Aerosol Lidar and Infrared Pathfinder satellite Observation (CALIPSO) mission and extinction profiles from the Stratospheric Aerosol and Gas Experiment (SAGE) have been used to infer the spatial and temporal distributions of the ATAL since the late 90's. We found that aerosol optical thickness between 13-18km have increased by a factor of 2-3 over the past 16 years likely related to raising pollution levels in South East Asia occuring during the same period. Modelling studies of the ATAL using WACCAM 3 and GEOS-Chem have provided conflicting information on its origin and a better representation of in-cloud SO2 and aerosol lifetime in GOES-Chem seems to be key to obtain consistent results with the few SO2 measurements available in the UTLS during the Asian Monsoon. In situ measurements of aerosol and trace gases in the UTLS from several balloon campaigns which took place in summer 2014 and 2015 in Asia will be presented and discussed with combined satellite and modelling analysis.

  19. Retrieval of high-spectral-resolution lidar for atmospheric aerosol optical properties profiling

    NASA Astrophysics Data System (ADS)

    Liu, Dong; Luo, Jing; Yang, Yongying; Cheng, Zhongtao; Zhang, Yupeng; Zhou, Yudi; Duan, Lulin; Su, Lin

    2015-10-01

    High-spectral-resolution lidars (HSRLs) are increasingly being developed for atmospheric aerosol remote sensing applications due to the straightforward and independent retrieval of aerosol optical properties without reliance on assumptions about lidar ratio. In HSRL technique, spectral discrimination between scattering from molecules and aerosol particles is one of the most critical processes, which needs to be accomplished by means of a narrowband spectroscopic filter. To ensure a high retrieval accuracy of an HSRL system, the high-quality design of its spectral discrimination filter should be made. This paper reviews the available algorithms that were proposed for HSRLs and makes a general accuracy analysis of the HSRL technique focused on the spectral discrimination, in order to provide heuristic guidelines for the reasonable design of the spectral discrimination filter. We introduce a theoretical model for retrieval error evaluation of an HSRL instrument with general three-channel configuration. Monte Carlo (MC) simulations are performed to validate the correctness of the theoretical model. Results from both the model and MC simulations agree very well, and they illustrate one important, although not well realized fact: a large molecular transmittance and a large spectral discrimination ratio (SDR, i.e., ratio of the molecular transmittance to the aerosol transmittance) are beneficial t o promote the retrieval accuracy. The application of the conclusions obtained in this paper in the designing of a new type of spectroscopic filter, that is, the field-widened Michelson interferometer, is illustrated in detail. These works are with certain universality and expected to be useful guidelines for HSRL community, especially when choosing or designing the spectral discrimination filter.

  20. Lidar observations of high-altitude aerosol layers (cirrus clouds)

    NASA Astrophysics Data System (ADS)

    Deleva, Atanaska D.; Grigorov, Ivan V.

    2013-03-01

    Aerosols, clouds and aerosol-cloud interactions are recognized as the key factors influencing the climate. Clouds are the primary modulators of the Earth's radiative budget. This paper focuses on the detection of high-altitude aerosol layers in the troposphere over mid-latitude lidar station in Sofia, Bulgaria. They are situated in the height-region 6 km÷16 km, with thickness in the range 0.2 km÷5 km and have varying optical characteristics. On the basis of the general utilized classification of the Cirrus clouds, high values of the calculated atmospheric backscatter coefficient and Angströmexponent estimation results we conclude that the registered strongly scattered aerosol layers are Cirrus clouds. Lidar measurements are performed with an aerosol lidar, equipped with Nd:YAG laser at wavelengths 532 nm and 1064 nm. Mainly, lidar data are presented in terms of vertical atmospheric backscatter coefficient profiles. We also include 2Dcolormap in height-time coordinates build on the basis of so called range corrected signals. It shows in general changes of the aerosol stratification over the lidar station during the measurement period. We employed HYSPLIT backward trajectories and DREAM forecasts to analyze the lidar profile outlines and characterize the events during which Cirrus cloud samples were observed. So was remarked that most of the results were obtained during Saharan dust long-way transport over the city of Sofia. Reported experimental examples are extracted from regular lidar investigations of the atmosphere within the frame of European project EARLINET.

  1. CNR-IMAA lidar systems for aerosol, clouds, and water vapour study

    NASA Astrophysics Data System (ADS)

    Pappalardo, G.; Amodeo, A.; Boselli, A.; Cornacchia, C.; D'Amico, G.; Madonna, F.; Mona, L.; Pandolfi, M.

    2005-10-01

    At CNR-IMAA located in Tito Scalo (40°36'N, 15°44'E, 760 m a.s.l.), two lidar systems are systematically operational: the first is devoted to tropospheric aerosol characterization, in the framework of EARLINET, and the second performs water vapour measurements. The aerosol lidar system provides independent measurements of aerosol extinction and backscatter coefficient at 355 nm and at 532 nm, aerosol backscatter profiles at 1064 nm and particles depolarization ratio at 532 nm. The Raman lidar for the water vapor allows the vertical profiling of the water vapour mixing ratio with high spatial and temporal resolution up to the tropopause. The system has been calibrated by means of intensive measurement campaign of simultaneous and co-located radiosonde launches. CNR-IMAA is also provided with a DIAL mobile system for pollutants 3-dimensional spatial distribution. Besides these lidar systems, the CNR-IMAA ground based facility for Earth Observation includes ancillary instruments: a radiosounding system for PTU, ozone and wind measurements; a Sun photometer operative since December 2004 in the framework of AERONET; a 12 channels microwave radiometer for continuous measurements of temperature, relative humidity and water vapor, operative since February 2004; a ceilometer for continuous cloud cover monitoring. Lidar systems together with these ancillary instruments make the CNR-IMAA a heavily instrumented experimental site for integrated observations of aerosols, clouds and water vapor to be used for climatological studies and for the validation of satellite data.

  2. Retrieving the height of smoke and dust aerosols by synergistic use of VIIRS, OMPS, and CALIOP observations

    NASA Astrophysics Data System (ADS)

    Lee, Jaehwa; Hsu, N. Christina; Bettenhausen, Corey; Sayer, Andrew M.; Seftor, Colin J.; Jeong, Myeong-Jae

    2015-08-01

    This study extends the application of the previously developed Aerosol Single-scattering albedo and layer Height Estimation (ASHE) algorithm, which was originally applied to smoke aerosols only, to both smoke and dust aerosols by including nonspherical dust properties in the retrieval process. The main purpose of the algorithm is to derive aerosol height information over wide areas using aerosol products from multiple satellite sensors simultaneously: aerosol optical depth (AOD) and Ångström exponent from the Visible Infrared Imaging Radiometer Suite (VIIRS), UV aerosol index from the Ozone Mapping and Profiler Suite (OMPS), and total backscatter coefficient profile from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). The case studies suggest that the ASHE algorithm performs well for both smoke and dust aerosols, showing root-mean-square error of the retrieved aerosol height as compared to CALIOP observations from 0.58 to 1.31 km and mean bias from -0.70 to 1.13 km. In addition, the algorithm shows the ability to retrieve single-scattering albedo to within 0.03 of Aerosol Robotic Network inversion data for moderate to thick aerosol loadings (AOD of ~1.0). For typical single-layered aerosol cases, the estimated uncertainty in the retrieved height ranges from 1.20 to 1.80 km over land and from 1.15 to 1.58 km over ocean when favorable conditions are met. Larger errors are observed for multilayered aerosol events, due to the limited sensitivities of the passive sensors to such cases.

  3. Lidar Observations of Tropospheric Aerosols Over Northeastern South Africa During the ARREX and SAFARI-2000 Dry Season Experiments

    NASA Technical Reports Server (NTRS)

    Campbell, James R.; Welton, Ellsworth J.; Spinhirne, James D.; Ji, Qiang; Tsay, Si-Chee; Piketh, Stuart J.; Barenbrug, Marguerite; Holben, Brent; Starr, David OC. (Technical Monitor)

    2002-01-01

    During the ARREX-1999 and SAFARI-2000 Dry Season experiments a micropulse lidar (523 nm) instrument was operated at the Skukuza Airport in northeastern South Africa. The Mar was collocated with a diverse array of passive radiometric equipment. For SAFARI-2000 the processed Mar data yields a daytime time-series of layer mean/derived aerosol optical properties, including extinction-to-backscatter ratios and vertical extinction cross-section profile. Combined with 523 run aerosol optical depth and spectral Angstrom exponent calculations from available CIMEL sun-photometer data and normalized broadband flux measurements the temporal evolution of the near surface aerosol layer optical properties is analyzed for climatological trends. For the densest smoke/haze events the extinction-to-backscatter ratio is found to be between 60-80/sr, and corresponding Angstrom exponent calculations near and above 1.75. The optical characteristics of an evolving smoke event from SAFARI-2000 are extensively detailed. The advecting smoke was embedded within two distinct stratified thermodynamic layers, causing the particulate mass to advect over the instrument array in an incoherent manner on the afternoon of its occurrence. Surface broadband flux forcing due to the smoke is calculated, as is the evolution in the vertical aerosol extinction profile as measured by the Han Finally, observations of persistent elevated aerosol during ARREX-1999 are presented and discussed. The lack of corroborating observations the following year makes these observation; both unique and noteworthy in the scope of regional aerosol transport over southern Africa.

  4. Comparison of Aerosol Optical Properties and Water Vapor Among Ground and Airborne Lidars and Sun Photometers During TARFOX

    NASA Technical Reports Server (NTRS)

    Ferrare, R.; Ismail, S.; Browell, E.; Brackett, V.; Clayton, M.; Kooi, S.; Melfi, S. H.; Whiteman, D.; Schwemmer, G.; Evans, K.; Russell, P.; Livingston, J.; Schmid, B.; Holben, B.; Remer, L.; Smirnov, A.; Hobbs, P. V.

    2000-01-01

    We compare aerosol optical thickness (AOT) and precipitable water vapor (PWV) measurements derived from ground and airborne lidars and Sun photometers during TARFOX (Tropospheric Aerosol Radiative Forcing Observational Experiment). Such comparisons are important to verify the consistency between various remote sensing measurements before employing them in any assessment of the impact of aerosols on the global radiation balance. Total scattering ratio and extinction profiles measured by the ground-based NASA/GSFC Scanning Raman Lidar (SRL) system, which operated from Wallops Island, Virginia (37.86 deg N, 75.51 deg W), are compared with those measured by the Lidar Atmospheric Sensing Experiment (LASE) airborne lidar system aboard the NASA ER-2 aircraft. Bias and rms differences indicate that these measurements generally agreed within about 10%. Aerosol extinction profiles and estimates of AOT are derived from both lidar measurements using a value for the aerosol extinction/backscattering ratio S(sub a)=60 sr for the aerosol extinction/backscattering ratio, which was determined from the Raman lidar measurements.

  5. Evaluation of regional air quality models in the presence of moderate to strong aerosol events

    NASA Astrophysics Data System (ADS)

    O'Neill, N. T.; Thulasiraman, S.; Pancrati, O.; Aube, M.; Lupu, A.; Neary, L.; Strawbridge, K.; Freemantle, J.; Kaminski, J.; McConnell, J.

    2006-12-01

    During the 2004 to 2006 period a program of synchronized sunphotometry and lidar backscatter measurements were carried out at Egbert, Ontario (70 km north of Toronto). A variety of events, ranging from moderate to strong pollution events, long and short distance smoke transport, long distance dust transport and the presence of thin homogeneous clouds were registered and optically analyzed. These data were employed to help evaluate the performance of the Canadian GEM-AQ air quality model as well an aerosol optical assimilation model (NOMAD). The evaluations were based on optical indicators of integrated aerosol content (aerosol optical depth), particle size indicators such as Angstrom exponent, and vertical profiles of the aerosol backscatter ratio. Some preliminary analyses will be presented; the focus will be on the problems associated with emissions modelling, the influence of cloud screening algorithms in the data and in the model, the robustness of particle size information in the passive optical data and the ability of the models to capture subtle variations, and the vertical performance of the models relative to the lidar backscatter data.

  6. Seasonal Variations in Titan's Stratosphere Observed with Cassini/CIRS: Temperature, Trace Molecular Gas and Aerosol Mixing Ratio Profiles

    NASA Technical Reports Server (NTRS)

    Vinatier, S.; Bezard, B.; Anderson, C. M.; Coustenis, A.; Teanby, N.

    2012-01-01

    Titan's northern spring equinox occurred in August 2009. General Circulation Models (e.g. Lebonnois et al., 2012) predict strong modifications of the global circulation in this period, with formation of two circulation cells instead of the pole-to-pole cell that occurred during northern winter. This winter single cell, which had its descending branch at the north pole, was at the origin of the enrichment of molecular abundances and high stratopause temperatures observed by Cassini/CIRS at high northern latitudes (e.g. Achterberg et al., 2011, Coustenis et al., 2010, Teanby et al., 2008, Vinatier et al., 2010). The predicted dynamical seasonal variations after the equinox have strong impact on the spatial distributions of trace gas, temperature and aerosol abundances. We will present here an analysis of CIRS limb-geometry datasets acquired in 2010 and 2011 that we used to monitor the seasonal evolution of the vertical profiles of temperature, molecular (C2H2, C2H6, HCN, ..) and aerosol abundances.

  7. HARLIE 3-D Aerosol Backscatter and Wind Profile Measurements During Recent Field Experiments: Background Noise Reduction with a Fabry-Perot Etalon Filter in the HARLIE System

    NASA Technical Reports Server (NTRS)

    Lee, Sangwoo; Miller, David O.; Schwemmer, Geary; Wilkerson, Thomas D.; Andrus, Ionio; Egbert, Cameron; Anderson, Mark; Starr, David OC. (Technical Monitor)

    2002-01-01

    Background noise reduction of War signals is one of the most important factors in achieving better signal to noise ratio and precise atmospheric data from Mar measurements. Fahey Perot etalons have been used in several lidar systems as narrow band pass filters in the reduction of scattered sunlight. An slalom with spectral bandwidth, (Delta)v=0.23/cm, free spectral range, FSR=6.7/cm, and diameter, d=24mm was installed in a fiber coupled box which included a 500 pm bandwidth interference Filter. The slalom box couples the telescope and detector with 200 pm core fibers and 21 mm focal length collimators. The angular magnification is M=48. The etalon box was inserted into the Holographic Airborne Rotating Lidar Instrument Experiment (HARLIE) system and tested during the HARGLO-2 intercomparison campaign conducted in November 2001 at Wallops Island, Virginia. This paper presents the preliminary test results of the slalom and a complete analysis will be presented at the conference.

  8. Extracting electron backscattering coefficients from backscattered electron micrographs

    SciTech Connect

    Zupanic, F.

    2010-12-15

    Electron backscattering micrographs possess the so-called Z-contrast, carrying information about the chemical compositions of phases present in microstructures. The intensity at a particular point in the backscattered electron micrograph is proportional to the signal detected at a corresponding point in the scan raster, which is, in turn, proportional to the electron backscattering coefficient of a phase at that point. This article introduces a simple method for extracting the electron backscattering coefficients of phases present in the microstructure, from the backscattered electron micrographs. This method is able to convert the micrograph's greyscale to the backscattering-coefficient-scale. The prerequisite involves the known backscattering coefficients for two phases in the micrograph. In this way, backscattering coefficients of other phases can be determined. The method is unable to determine the chemical compositions of phases or the presence of an element only from analysing the backscattered electron micrograph. Nevertheless, this method was found to be very powerful when combined with energy dispersive spectroscopy, and the calculations of backscattering coefficients. - Research Highlights: {yields}A simple method for extracting the electron backscattering coefficients {yields}The prerequisite is known backscattering coefficients for two phases {yields}The information is complementary to the EDS-results. {yields}This method is especially useful when a phase contains a light element (H, Li, Be, and B)

  9. Critical Evaluation of 0-30 km Profile Information in Ground-Based Zenith-Sky and Satellite-Measured Backscattered UV Radiation

    NASA Technical Reports Server (NTRS)

    Bhartia, Pawan; Petropavlovskikh, Irina; Deluishi, John; Einaudi, Franco (Technical Monitor)

    2000-01-01

    We now have several decades of experience in deriving vertical ozone profiles from the measurements of diffuse ultraviolet radiation by both ground and satellite-based instruments using Umkehr and BUV techniques. Continuing technological advances are pushing the state-of-the-art of these measurements to high spectral resolution and broader wavelength coverage. These modern instruments include the ground-based Brewer and satellite-based Global Ozone Monitoring Experiment (GOME) instruments, as well as advanced instruments being developed by ESA(SCIAMACHY), Netherlands(OMI) and Japan(ODUS). However, one of the issues that remains unresolved is the 0-30 km ozone profile information retrievable from these measurements. Though it is commonly believed that both the Umkehr and the satellite-based BUV techniques have very limited profile information below 30 km, there are those who argue that the data from these instruments should continue to be reported in this altitude range for they compare well with ozonesondes and hence there is useful scientific information. Others claim that the limitations of the Umkehr and BUV techniques are largely due to their low spectral resolution, and that the profile information below 30 km can be greatly improved by going to high spectral resolution instruments, such as Brewer and GOME. The purpose of this paper is to provide a critical evaluation of the 0-30 km ozone profile information in the various UV remote sensing techniques. We use a database of individual ozone profiles created using ozonesondes and SAGE and 4D ozone fields generated by data assimilation techniques to simulate radiances measured by the various techniques. We then apply a common inversion approach to all the methods to systematically examine how much profile information is available simply from the knowledge of total ozone, how much additional profile information is added by the traditional Dobson Umkehr and satellite buv techniques, and how much better one can do

  10. Lidar measurements of stratospheric aerosols over Menlo Park, California, October 1972 - March 1974

    NASA Technical Reports Server (NTRS)

    Russell, P. B.; Viezee, W.; Hake, R. D.

    1974-01-01

    During an 18-month period, 30 nighttime observations of stratospheric aerosols were made using a ground based ruby lidar located near the Pacific coast of central California (37.5 deg. N, 122.2 deg. W). Vertical profiles of the lidar scattering ratio and the particulate backscattering coefficient were obtained by reference to a layer of assumed negligible particulate content. An aerosol layer centered near 21 km was clearly evident in all observations, but its magnitude and vertical distribution varied considerably throughout the observation period. A reduction of particulate backscattering in the 23- to 30-km layer during late January 1973 appears to have been associated with the sudden stratospheric warming which occurred at that time.

  11. Reducing the uncertainty in background marine aerosol radiative properties using CAM5 model results and CALIPSO-retrievals

    NASA Astrophysics Data System (ADS)

    Meskhidze, N.; Gantt, B.; Dawson, K.; Johnson, M. S.; Gasso, S.

    2012-12-01

    Abundance of natural aerosols in the atmosphere strongly affects global aerosol optical depth (AOD) and influences clouds and the hydrological cycle through its ability to act as cloud condensation nuclei (CCN). Because the anthropogenic contribution to climate forcing represents the difference between the total forcing and that from natural aerosols, understanding background aerosols is necessary to evaluate the influences of anthropogenic aerosols on cloud reflectivity and persistence (so-called indirect radiative forcing). The effects of marine aerosols are explored using remotely sensed data obtained by Cloud-aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and the NCAR Community Atmosphere Model (CAM5.0), coupled with the PNNL Modal Aerosol Model. CALIPSO-provided high resolution vertical profile information about different aerosol subtypes (defined as clean continental, marine, desert dust, polluted continental, polluted dust, and biomass burning), particulate depolarization ratio (or particle non-sphericity), reported aerosol color ratio (the ratio of aerosol backscatter at the two wavelengths) and lidar ratios over different parts of the oceans are compared to model-simulations to help evaluate the contribution of biogenic aerosol to CCN budget in the marine boundary layer. Model-simulations show that over biologically productive ocean waters primary organic aerosols of marine origin can contribute up to a 20% increase in CCN (at a supersaturation of 0.2%) number concentrations. Corresponding changes associated with cloud properties (liquid water path and droplet number) can decrease global annual mean indirect radiative forcing of anthropogenic aerosol (less cooling) by ~0.1 Wm-2 (7%). This study suggests ignoring the complex chemical composition and size distribution of sea spray particles could result in considerable uncertainties in predicted anthropogenic aerosol indirect effect.

  12. Airborne water vapor DIAL system and measurements of water and aerosol profiles

    NASA Technical Reports Server (NTRS)

    Higdon, Noah S.; Browell, Edward V.

    1991-01-01

    The Lidar Applications Group at NASA Langley Research Center has developed a differential absorption lidar (DIAL) system for the remote measurement of atmospheric water vapor (H2O) and aerosols from an aircraft. The airborne H2O DIAL system is designed for extended flights to perform mesoscale investigations of H2O and aerosol distributions. This DIAL system utilizes a Nd:YAG-laser-pumped dye laser as the off-line transmitter and a narrowband, tunable Alexandrite laser as the on-line transmitter. The dye laser has an oscillator/amplifier configuration which incorporates a grating and prism in the oscillator cavity to narrow the output linewidth to approximately 15 pm. This linewidth can be maintained over the wavelength range of 725 to 730 nm, and it is sufficiently narrow to satisfy the off-line spectral requirements. In the Alexandrite laser, three intracavity tuning elements combine to produce an output linewidth of 1.1 pm. These spectral devices include a five-plate birefringent tuner, a 1-mm thick solid etalon and a 1-cm air-spaced etalon. A wavelength stability of +/- 0.35 pm is achieved by active feedback control of the two Fabry-Perot etalons using a frequency stabilized He-Ne laser as a wavelength reference. The three tuning elements can be synchronously scanned over a 150 pm range with microprocessor-based scanning electronics. Other aspects of the DIAL system are discussed.

  13. Size-time composition profile of aerosols using the drum sampler

    NASA Astrophysics Data System (ADS)

    Cahill, Thomas A.; Feeney, Patrick J.; Eldred, Robert A.

    1987-03-01

    Mie scattering theory imposes strict requirements for both size and compositional information on aerosols associated with visibility degradation. But, at the very clean National Park Service sites where we do such studies, episodes of degraded visibility may be infrequent and of short duration. To meet these needs, an 8 stage impactor of the Battelle/SFU design was mated to rotating drum impaction surfaces of the Lundgren design in a compact and rugged DRUM sampler of Davis design. This unit, three years in development, has been extensively tested using laboratory aerosols and field intercomparisons. The standard unit runs essentially unattended for 14 or 28 days. The samples are analyzed in 2 to 8 hour time segments. Analyses are done by carefully collimated (1 mm, 2 mm) proton beams in a tightly coupled PIXE system, yielding sensitivities of a few {solng}/{m 3}. Dramatic shifts in the size distribution of sulfur versus time have been observed, with direct influence on optical extinction. Further, primary smelter effluents have been clearly identified at Grand Canyon NP, but only in the < 0.15 μm size fraction. The DRUM sampler makes excellent use of PIXE capabilities, but can also be analyzed by lasers (Csoot) and β-gauging (mass).

  14. Impact of black carbon aerosol over Italian basin valleys: high-resolution measurements along vertical profiles, radiative forcing and heating rate

    NASA Astrophysics Data System (ADS)

    Ferrero, L.; Castelli, M.; Ferrini, B. S.; Moscatelli, M.; Perrone, M. G.; Sangiorgi, G.; D'Angelo, L.; Rovelli, G.; Moroni, B.; Scardazza, F.; Močnik, G.; Bolzacchini, E.; Petitta, M.; Cappelletti, D.

    2014-09-01

    A systematic study of black carbon (BC) vertical profiles measured at high-resolution over three Italian basin valleys (Terni Valley, Po Valley and Passiria Valley) is presented. BC vertical profiles are scarcely available in literature. The campaign lasted 45 days and resulted in 120 measured vertical profiles. Besides the BC mass concentration, measurements along the vertical profiles also included aerosol size distributions in the optical particle counter range, chemical analysis of filter samples and a full set of meteorological parameters. Using the collected experimental data, we performed calculations of aerosol optical properties along the vertical profiles. The results, validated with AERONET data, were used as inputs to a radiative transfer model (libRadtran). The latter allowed an estimation of vertical profiles of the aerosol direct radiative effect, the atmospheric absorption and the heating rate in the lower troposphere. The present measurements revealed some common behaviors over the studied basin valleys. Specifically, at the mixing height, marked concentration drops of both BC (range: from -48.4 ± 5.3 to -69.1 ± 5.5%) and aerosols (range: from -23.9 ± 4.3 to -46.5 ± 7.3%) were found. The measured percentage decrease of BC was higher than that of aerosols: therefore, the BC aerosol fraction decreased upwards. Correspondingly, both the absorption and scattering coefficients decreased strongly across the mixing layer (range: from -47.6 ± 2.5 to -71.3 ± 3.0% and from -23.5 ± 0.8 to -61.2 ± 3.1%, respectively) resulting in a single-scattering albedo increase along height (range: from +4.9 ± 2.2 to +7.4 ± 1.0%). This behavior influenced the vertical distribution of the aerosol direct radiative effect and of the heating rate. In this respect, the highest atmospheric absorption of radiation was predicted below the mixing height (~ 2-3 times larger than above it) resulting in a heating rate characterized by a vertical negative gradient (range

  15. Polarization lidar returns from aerosols and thin clouds: a framework for the analysis.

    PubMed

    Gobbi, G P

    1998-08-20

    Relationships for the interpretation of polarization lidar observations of aerosols and thin clouds are presented. They allow for the separation of contributions to backscatter from solid and liquid phases by the use of either the classical backscatter and depolarization ratio parameters or the particulate cross-polarized backscatter cross sections. It is shown that different aerosol phases can be better separated by use of the latter coordinates. Emphasis is placed on the study of composition and phase properties of polar stratospheric aerosols.

  16. Vertical Profiles of Light-Absorbing Aerosol: A Combination of In-situ and AERONET Observations during NASA DISCOVER-AQ

    NASA Astrophysics Data System (ADS)

    Ziemba, L. D.; Beyersdorf, A. J.; Chen, G.; Corr, C.; Crumeyrolle, S.; Giles, D. M.; Holben, B. N.; Hudgins, C.; Martin, R.; Moore, R.; Shook, M.; Thornhill, K. L., II; Winstead, E.; Anderson, B. E.

    2014-12-01

    Understanding the vertical profile of atmospheric aerosols plays a vital role in utilizing spaceborne, column-integrated satellite observations. The properties and distribution of light-absorbing aerosol are particularly uncertain despite significant air quality and climate ramifications. Advanced retrieval algorithms are able to derive complex aerosol properties (e.g., wavelength-dependent absorption coefficient and single scattering albedo) from remote-sensing measurements, but quantitative relationships to surface conditions remain a challenge. Highly systematic atmospheric profiling during four unique deployments for the NASA DISCOVER-AQ project (Baltimore, MD, 2011; San Joaquin Valley, CA, 2013; Houston, TX, 2013; Denver, CO, 2014) allow statistical assessment of spatial, temporal, and source-related variability for light-absorbing aerosol properties in these distinct regions. In-situ sampling in conjunction with a dense network of AERONET sensors also allows evaluation of the sensitivity, limitations, and advantages of remote-sensing data products over a wide range of conditions. In-situ aerosol and gas-phase observations were made during DISCOVER-AQ aboard the NASA P-3B aircraft. Aerosol absorption coefficients were measured by a Particle Soot Absorption Photometer (PSAP). Approximately 200 profiles for each of the four deployments were obtained, from the surface (25-300m altitude) to 5 km, and are used to calculate absorption aerosol optical depths (AAODs). These are quantitatively compared to AAOD derived from AERONET Level 1.5 retrievals to 1) explore discrepancies between measurements, 2) quantify the fraction of AAOD that exists directly at the surface and is often missed by airborne sampling, and 3) evaluate the potential for deriving ground-level black carbon (BC) concentrations for air quality prediction. Aerosol size distributions are used to assess absorption contributions from mineral dust, both at the surface and aloft. SP2 (Single Particle Soot

  17. Aerosol profiling with lidar in the Amazon Basin during the wet and dry season

    NASA Astrophysics Data System (ADS)

    Baars, H.; Ansmann, A.; Althausen, D.; Engelmann, R.; Heese, B.; Müller, D.; Artaxo, P.; Paixao, M.; Pauliquevis, T.; Souza, R.

    2012-11-01

    For the first time, multiwavelength polarization Raman lidar observations of optical and microphysical particle properties over the Amazon Basin are presented. The fully automated advanced Raman lidar was deployed 60 km north of Manaus, Brazil (2.5°S, 60°W) in the Amazon rain forest from January to November 2008. The measurements thus cover both the wet season (Dec-June) and the dry or burning season (July-Nov). Two cases studies of young and aged smoke plumes are discussed in terms of spectrally resolved optical properties (355, 532, and 1064 nm) and further lidar products such as particle effective radius and single-scattering albedo. These measurement examples confirm that biomass burning aerosols show a broad spectrum of optical, microphysical, and chemical properties. The statistical analysis of the entire measurement period revealed strong differences between the pristine wet and the polluted dry season. African smoke and dust advection frequently interrupt the pristine phases during the wet season. Compared to pristine wet season conditions, the particle scattering coefficients in the lowermost 2 km of the atmosphere were found to be enhanced, on average, by a factor of 4 during periods of African aerosol intrusion and by a factor of 6 during the dry (burning) season. Under pristine conditions, the particle extinction coefficients and optical depth for 532 nm wavelength were frequently as low as 10-30 Mm-1 and <0.05, respectively. During the dry season, biomass burning smoke plumes reached to 3-5 km height and caused a mean optical depth at 532 nm of 0.26. On average during that season, particle extinction coefficients (532 nm) were of the order of 100 Mm-1 in the main pollution layer (up to 2 km height). Ångström exponents were mainly between 1.0 and 1.5, and the majority of the observed lidar ratios were between 50-80 sr.

  18. Aerosol profiling with lidar in the Amazon Basin during the wet and dry season

    NASA Astrophysics Data System (ADS)

    Baars, H.; Ansmann, A.; Althausen, D.; Engelmann, R.; Heese, B.; Müller, D.; Artaxo, P.; Paixao, M.; Pauliquevis, T.; Souza, R.

    2011-11-01

    For the first time, multiwavelength polarization Raman lidar observations of optical and microphysical particle properties over the Amazon Basin are presented. The fully automated advanced Raman lidar was deployed 60 km north of Manaus, Brazil (2.5°S, 60°W) in the Amazon rain forest from January to November 2008. The measurements thus cover both the wet season (Dec-June) and the dry or burning season (July-Nov). Two cases studies of young and aged smoke plumes are discussed in terms of spectrally resolved optical properties (355, 532, and 1064 nm) and further lidar products such as particle effective radius and single-scattering albedo. These measurement examples confirm that biomass burning aerosols show a broad spectrum of optical, microphysical, and chemical properties. The statistical analysis of the entire measurement period revealed strong differences between the pristine wet and the polluted dry season. African smoke and dust advection frequently interrupt the pristine phases during the wet season. Compared to pristine wet season conditions, the particle scattering coefficients in the lowermost 2 km of the atmosphere were found to be enhanced, on average, by a factor of 4 during periods of African aerosol intrusion and by a factor of 6 during the dry (burning) season. Under pristine conditions, the particle extinction coefficients and optical depth for 532 nm wavelength were frequently as low as 10-30 Mm-1 and <0.05, respectively. During the dry season, biomass burning smoke plumes reached to 3-5 km height and caused a mean optical depth at 532 nm of 0.26. On average during that season, particle extinction coefficients (532 nm) were of the order of 100 Mm-1 in the main pollution layer (up to 2 km height). Ångström exponents were mainly between 1.0 and 1.5, and the majority of the observed lidar ratios were between 50-80 sr.

  19. Scanning Mobile Lidar for Aerosol Tracking and Biological Aerosol Identification

    NASA Astrophysics Data System (ADS)

    He, Tingyao; Bergant, Klemen; Filipčič, Andrej; Forte, Biagio; Gao, Fei; Stanič, Samo; Veberič, Darko; Zavrtanik, Marko

    2010-05-01

    Optical properties of non-biological aerosols containing aromatic hydrocarbons, such as industrial chemicals and engine exhausts, have already been thoroughly studied using remote sensing techniques. However, because of their complex composition and characteristics, the identification of biological aerosols, such as fungi, pollen and bacteria that are present in the environment remains a rather difficult task. The collection of information on both non-biological and biological aerosols is of great importance for understanding their interrelation, physical and chemical properties and their influence on human health and the environment. Biological and non-biological aerosols can be simultaneously detected, tracked and identified by a scanning mobile Mie-fluorescence lidar. The device developed at the University of Nova Gorica can perform azimuth and zenith angle scans with an angular resolution of 0.1°, as well as operate in both day and night-time conditions. Aerosols of biological origin are identified through the detection of the fluorescence of the amino acid tryptophan which is present in almost all substances of biological origin. In our system, the transmitter is a solid state Nd:YAG laser which is capable of simultaneous emission of light at a base wavelength of 1064 nm (IR) and its quadrupled wavelength of 266 nm (UV) at a maximum repetition rate of 10 Hz. Tryptophan contained in biological aerosols is excited by the 266 nm laser pulses and the returning fluorescence signals are detected in the spectral band centered at 295 nm. The receiver is a Newtonian telescope which uses a 300 mm parabolic mirror to direct received light into three detection channels - two elastic backscatter channels (IR and UV) and a fluorescence channel. First experiments show that the detection range of the lidar reaches 10 km in the IR channel and 3 km in the UV channel. Based on the preliminary simulations of the signal-to-noise ratio, the detection range for biological

  20. A statistical inference approach for the retrieval of the atmospheric ozone profile from simulated satellite measurements of solar backscattered ultraviolet radiation

    NASA Technical Reports Server (NTRS)

    Bonavito, N. L.; Gordon, C. L.; Inguva, R.; Serafino, G. N.; Barnes, R. A.

    1994-01-01

    NASA's Mission to Planet Earth (MTPE) will address important interdisciplinary and environmental issues such as global warming, ozone depletion, deforestation, acid rain, and the like with its long term satellite observations of the Earth and with its comprehensive Data and Information System. Extensive sets of satellite observations supporting MTPE will be provided by the Earth Observing System (EOS), while more specific process related observations will be provided by smaller Earth Probes. MTPE will use data from ground and airborne scientific investigations to supplement and validate the global observations obtained from satellite imagery, while the EOS satellites will support interdisciplinary research and model development. This is important for understanding the processes that control the global environment and for improving the prediction of events. In this paper we illustrate the potential for powerful artificial intelligence (AI) techniques when used in the analysis of the formidable problems that exist in the NASA Earth Science programs and of those to be encountered in the future MTPE and EOS programs. These techniques, based on the logical and probabilistic reasoning aspects of plausible inference, strongly emphasize the synergetic relation between data and information. As such, they are ideally suited for the analysis of the massive data streams to be provided by both MTPE and EOS. To demonstrate this, we address both the satellite imagery and model enhancement issues for the problem of ozone profile retrieval through a method based on plausible scientific inferencing. Since in the retrieval problem, the atmospheric ozone profile that is consistent with a given set of measured radiances may not be unique, an optimum statistical method is used to estimate a 'best' profile solution from the radiances and from additional a priori information.

  1. Investigation of wintertime cold-air pools and aerosol layers in the Salt Lake Valley using a lidar ceilometer

    NASA Astrophysics Data System (ADS)

    Young, Joseph Swyler

    This thesis investigates the utility of lidar ceilometers, a type of aerosol lidar, in improving the understanding of meteorology and air quality in persistent wintertime stable boundary layers, or cold-air pools, that form in urbanized valley and basin topography. This thesis reviews the scientific literature to survey the present knowledge of persistent cold-air pools, the operating principles of lidar ceilometers, and their demonstrated utility in meteorological investigations. Lidar ceilometer data from the Persistent Cold-Air Pool Study (PCAPS) are then used with meteorological and air quality data from other in situ and remote sensing equipment to investigate cold-air pools that formed in Utah's Salt Lake Valley during the winter of 2010-2011. The lidar ceilometer is shown to accurately measure aerosol layer depth and aerosol loading, when compared to visual observations. A linear relationship is found between low-level lidar backscatter and surface particulate measurements. Convective boundary layer lidar analysis techniques applied to cold-air pool ceilometer profiles can detect useful layer characteristics. Fine-scale waves are observed and analyzed within the aerosol layer, with emphasis on Kelvin-Helmholz waves. Ceilometer aerosol backscatter profiles are analyzed to quantify and describe mixing processes in persistent cold-air pools. Overlays of other remote and in-situ observations are combined with ceilometer particle backscatter to describe specific events during PCAPS. This analysis describes the relationship between the aerosol layer and the valley inversion as well as interactions with large-scale meteorology. The ceilometer observations of hydrometers are used to quantify cloudiness and precipitation during the project, observing that 50% of hours when a PCAP was present had clouds or precipitation below 5 km above ground level (AGL). Then, combining an objective technique for determining hourly aerosol layer depths and correcting this

  2. THERMAL NEUTRON BACKSCATTER IMAGING.

    SciTech Connect

    VANIER,P.; FORMAN,L.; HUNTER,S.; HARRIS,E.; SMITH,G.

    2004-10-16

    Objects of various shapes, with some appreciable hydrogen content, were exposed to fast neutrons from a pulsed D-T generator, resulting in a partially-moderated spectrum of backscattered neutrons. The thermal component of the backscatter was used to form images of the objects by means of a coded aperture thermal neutron imaging system. Timing signals from the neutron generator were used to gate the detection system so as to record only events consistent with thermal neutrons traveling the distance between the target and the detector. It was shown that this time-of-flight method provided a significant improvement in image contrast compared to counting all events detected by the position-sensitive {sup 3}He proportional chamber used in the imager. The technique may have application in the detection and shape-determination of land mines, particularly non-metallic types.

  3. Radar backscatter modelling

    NASA Technical Reports Server (NTRS)

    Schaber, G. G.; Kozak, R. C.; Gurule, R. L.

    1984-01-01

    The terrain analysis software package was restructured and documentation was added. A program was written to test Johnson Space Center's four band scatterometer data for spurious signals data. A catalog of terrain roughness statistics and calibrated four frequency multipolarization scatterometer data is being published to support the maintenance of Death Valley as a radar backscatter calibration test site for all future airborne and spacecraft missions. Test pits were dug through sand covered terrains in the Eastern Sahara to define the depth and character of subsurface interfaces responsible for either backscatter or specular response in SIR-A imagery. Blocky sandstone bedrock surfaces at about 1 m depth were responsible for the brightest SIR-A returns. Irregular very dense CaCO3 cemented sand interfaces were responsible for intermediate grey tones. Ancient river valleys had the weakest response. Reexamination of SEASAT l-band imagery of U.S. deserts continues.

  4. Development of global model for atmospheric backscatter at CO2 wavelengths

    NASA Technical Reports Server (NTRS)

    Kent, G. S.; Wang, P. H.; Farrukh, U.; Deepak, A.; Patterson, E. M.

    1985-01-01

    The improvement of an understanding of the variation of the aerosol backscattering at 10.6 micron within the free troposphere and the development model to describe this was undertaken. The analysis combines theoretical modeling with the results contained within three independent data sets. The data sets are obtained by the SAGE I/SAM II satellite experiments, the GAMETAG flight series and by direct backscatter measurements. The theoretical work includes use of a bimodal, two component aerosol model, and the study of the microphysical and associated optical changes occurring within an aerosol plume. A consistent picture is obtained, which describes the variation of the aerosol backscattering function in the free troposphere with altitude, latitude, and season. Most data are available and greatest consistency is found inside the Northern Hemisphere.

  5. Development of a global model for atmospheric backscatter at CO2 wavelengths

    NASA Technical Reports Server (NTRS)

    Kent, G. S.; Wang, P. H.; Farrukh, U.; Deepak, A.; Patterson, E. M.

    1986-01-01

    The variation of the aerosol backscattering at 10.6 micrometers within the free troposphere was investigated and a model to describe this variation was developed. The analysis combines theoretical modeling with the results contained within three independent data sets. The data sets used were obtained by the SAGE I/SAM II satellite experiments, the GAMETAG flight series, and by direct backscatter measurements. The theoretical work includes use of a bimodal, two component aerosol model, and the study of the microphysical and associated optical changes occurring within an aerosol plume. A consistent picture is obtained that describes the variation of the aerosol backscattering function in the free troposphere with altitude, latitude, and season.

  6. Dependence of the drizzle growth process on the cloud top height and its relevance to the aerosol vertical profile

    NASA Astrophysics Data System (ADS)

    Kawamoto, K.; Suzuki, K.

    2013-12-01

    Transitional processes among cloud droplets, drizzle and raindrops are still uncertain and more efforts are required for the better understanding. In this situation, difference in the drizzle growth process was examined according to the cloud top height using the CloudSat and MODIS synergetic datasets. From the CloudSat products such as 2B-GEOPROF, 2B-TAU, ECMWF-AUX, only one-layered water clouds whose top temperatures were warmer than 273K were extracted over China (a circular area having a diameter of 1800km of the center at 35°N and 120°E) and over ocean (a circular area having a diameter of 1500km of the center at 35°N and 150°E). Then a threshold of 3km of the cloud top height was adopted to divide the extracted clouds into upper and lower cases. First, the probability distribution functions (PDF) of the cloud droplet number density (Nc) and the effective particle radius (Re) were calculated for these four cases (land/ocean/upper/lower). Nc was obtained assuming the adiabatic liquid water content from MODIS-derived cloud optical depth and Re. Oceanic clouds had fewer Nc than land clouds, and almost the same for upper and lower cases. Land clouds had more Nc for the lower case than for the higher case. On the other hand, oceanic clouds had larger Re than land clouds, and almost the same for upper and lower cases. Land clouds had smaller Re for the lower case than for the higher case. These results quite agreed with our existing knowledge on the vertical profile of the aerosol number concentration over ocean (pristine) and land (polluted). Although the number of aerosol particles is fewer and almost the same regardless of the height over the ocean, it is more near the surface and it rapidly decreases according to the height over the land. Next, examining PDF of the radar reflectivity (Ze), we found that although PDFs of Ze were almost the same for oceanic clouds regardless of the cloud top height, PDF of land lower clouds were less frequent at around from

  7. A method for removing arm backscatter from EPID images

    SciTech Connect

    King, Brian W.; Greer, Peter B.

    2013-07-15

    Purpose: To develop a method for removing the support arm backscatter from images acquired using current Varian electronic portal imaging devices (EPIDs).Methods: The effect of arm backscatter on EPID images was modeled using a kernel convolution method. The parameters of the model were optimized by comparing on-arm images to off-arm images. The model was used to develop a method to remove the effect of backscatter from measured EPID images. The performance of the backscatter removal method was tested by comparing backscatter corrected on-arm images to measured off-arm images for 17 rectangular fields of different sizes and locations on the imager. The method was also tested using on- and off-arm images from 42 intensity modulated radiotherapy (IMRT) fields.Results: Images generated by the backscatter removal method gave consistently better agreement with off-arm images than images without backscatter correction. For the 17 rectangular fields studied, the root mean square difference of in-plane profiles compared to off-arm profiles was reduced from 1.19% (standard deviation 0.59%) on average without backscatter removal to 0.38% (standard deviation 0.18%) when using the backscatter removal method. When comparing to the off-arm images from the 42 IMRT fields, the mean {gamma} and percentage of pixels with {gamma} < 1 were improved by the backscatter removal method in all but one of the images studied. The mean {gamma} value (1%, 1 mm) for the IMRT fields studied was reduced from 0.80 to 0.57 by using the backscatter removal method, while the mean {gamma} pass rate was increased from 72.2% to 84.6%.Conclusions: A backscatter removal method has been developed to estimate the image acquired by the EPID without any arm backscatter from an image acquired in the presence of arm backscatter. The method has been shown to produce consistently reliable results for a wide range of field sizes and jaw configurations.

  8. Influence of atmospheric parameters on vertical profiles and horizontal transport of aerosols generated in the surf zone

    NASA Astrophysics Data System (ADS)

    Kusmierczyk-Michulec, J.; Tedeschi, G.; Van Eijk, A. M. J.; Piazzola, J.

    2013-10-01

    The vertical and horizontal transport of aerosols generated over the surf zone is discussed. Experimental data were collected during the second campaign of the Surf Zone Aerosol Experiment that took place in Duck NC (USA) in November 2007. The Empirical Orthogonal Function (EOF) method was used to analyze the vertical concentration gradients, and allowed separating the surf aerosols from aerosols advected from elsewhere. The numerical Marine Aerosol Concentration Model (MACMod) supported the analysis by confirming that the concentration gradients are more pronounced under stable conditions and that aerosol plumes are then more confined to the surface. The model also confirmed the experimental observations made during two boat runs along the offshore wind vector that surf-generated aerosols are efficiently advected out to sea over several tens of kilometers.

  9. Space Borne Cloud and Aerosol Measurements by the Geoscience Laser Altimeter System: Initial Results

    NASA Technical Reports Server (NTRS)

    Spinhirne, James D.; Palm, Steven P.; Hlavka, Dennis L.; Hart, William D.; Mahesh, Ashwin; Welton, Ellsworth J.

    2003-01-01

    In January 2003 the Geoscience Laser Altimeter System (GLAS) was successfully launched into orbit. Beginning in March 2003 GLAS will provide global coverage lidar measurement of the height distribution of clouds and aerosol in the atmosphere for up to five years. The characteristic and value of the unique data will be presented. The instrument is a basic backscatter lidar that operates at two wavelengths, 532 and 1064 nm. The mission data products for atmospheric observations include the calibrated, observed, attenuated backscatter cross section for cloud and aerosol; height detection for multiple cloud layers; planetary boundary layer height; cirrus and aerosol optical depth and the height distribution of aerosol and cloud scattering cross section profiles. The data is expected to significantly enhance knowledge in several areas of atmospheric science, in particular the distribution, transport and influence of atmospheric aerosol and thin clouds. Measurements of the coverage and height of polar and cirrus cloud should be significantly more accurate than previous global observations. In March and April 2003, airborne and ground based data verification experiments will be carried out. Initial results from the verification experiments and the first several months of operation will be presented.

  10. Vertical distribution of aerosol optical properties based on aircraft measurements over the Loess Plateau in China.

    PubMed

    Li, Junxia; Liu, Xingang; Yuan, Liang; Yin, Yan; Li, Zhanqing; Li, Peiren; Ren, Gang; Jin, Lijun; Li, Runjun; Dong, Zipeng; Li, Yiyu; Yang, Junmei

    2015-08-01

    Vertical distributions of aerosol optical properties based on aircraft measurements over the Loess Plateau were measured for the first time during a summertime aircraft campaign, 2013 in Shanxi, China. Data from four flights were analyzed. The vertical distributions of aerosol optical properties including aerosol scattering coefficients (σsc), absorption coefficients (σab), Angström exponent (α), single scattering albedo (ω), backscattering ratio (βsc), aerosol mass scattering proficiency (Qsc) and aerosol surface scattering proficiency (Qsc(')) were obtained. The mean statistical values of σsc were 77.45 Mm(-1) (at 450 nm), 50.72 Mm(-1) (at 550n m), and 32.02 Mm(-1) (at 700 nm). The mean value of σab was 7.62 Mm(-1) (at 550 nm). The mean values of α, βsc and ω were 1.93, 0.15, and 0.91, respectively. Aerosol concentration decreased with altitude. Most effective diameters (ED) of aerosols were less than 0.8 μm. The vertical profiles of σsc,, α, βsc, Qsc and Qsc(') showed that the aerosol scattering properties at lower levels contributed the most to the total aerosol radiative forcing. Both α and βsc had relatively large values, suggesting that most aerosols in the observational region were small particles. The mean values of σsc, α, βsc, Qsc, Qsc('), σab and ω at different height ranges showed that most of the parameters decreased with altitude. The forty-eight hour backward trajectories of air masses during the observation days indicated that the majority of aerosols in the lower level contributed the most to the total aerosol loading, and most of these particles originated from local or regional pollution emissions.

  11. Ground-Based Lidar Measurements of Aerosols During ACE-2 Instrument Description, Results, and Comparisons with Other Ground-Based and Airborne Measurements

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth J.; Voss, Kenneth J.; Gordon, Howard R.; Maring, Hal; Smirnov, Alexander; Holben, Brent; Schmid, Beat; Livingston, John M.; Russell, Philip B.; Durkee, Philip A.; Formenti, Paolo

    2000-01-01

    A micro-pulse lidar system (MPL) was used to measure the vertical and horizontal distribution or aerosols during the Aerosol Characterization Experiment 2 (ACE-2) in June and July of 1997. The MPL measurements were made at the Izana observatory (IZO), a weather station located on a mountain ridge (28 deg 18'N, 16 deg 30'W, 2367 m asl) near the center of the island of Tenerife, Canary Islands. The MPL was used to acquire aerosol backscatter, extinction, and optical depth profiles for normal background periods and periods influenced by Saharan dust from North Africa. System tests and calibration procedures are discussed, and in analysis of aerosol optical profiles acquired during ACE-2 is presented. MPL data taken during normal IZO conditions (no dust) showed that upslope aerosols appeared during the day and dissipated at night and that the layers were mostly confined to altitudes a few hundred meters above IZO. MPL data taken during a Saharan dust episode on 17 July showed that peak aerosol extinction values were an order of magnitude greater than molecular scattering over IZO. and that the dust layers extended to 5 km asl. The value of the dust backscatter-extinction ratio was determined to be 0.027 + 0.007 per sr. Comparisons of the MPL data with data from other co-located instruments showed good agreement during the dust episode.

  12. Ground-Based Lidar Measurements of Aerosols During ACE-2: Instrument Description, Results, and Comparisons with Other Ground-Based and Airborne Measurements

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth J.; Voss, Kenneth J.; Gordon, Howard R.; Maring, Hal; Smirnov, Alexander; Holben, Brent; Schmid, Beat; Livingston, John M.; Russell, Philip B.; Durkee, Philip A.

    2000-01-01

    A micro-pulse lidar system (MPL) was used to measure the vertical and horizontal distribution of aerosols during the Aerosol Characterization Experiment 2 (ACE-2) in June and July of 1997. The MPL measurements were made at the Izana observatory (IZO), a weather station located on a mountain ridge (28 deg 18 min N, 16 deg 30 min W, 2367 m asl) near the center of the island of Tenerife, Canary Islands. The MPL was used to acquire aerosol backscatter, extinction, and optical depth profiles for normal background periods and periods influenced by Saharan dust from North Africa. System tests and calibration procedures are discussed, and an analysis of aerosol optical profiles acquired during ACE-2 is presented. MPL data taken during normal IZO conditions (no dust) showed that upslope aerosols appeared during the day and dissipated at night and that the layers were mostly confined to altitudes a few hundred meters above IZO. MPL data taken during a Saharan dust episode on 17 July showed that peak aerosol extinction values were an order of magnitude greater than molecular scattering over IZO, and that the dust layers extended to 5 km asl. The value of the dust backscatter-extinction ratio was determined to be 0.027 +/- 0.007 sr(exp -1). Comparisons of the MPL data with data from other collocated instruments showed good agreement during the dust episode.

  13. A Compact Mobile Ozone Lidar for Atmospheric Ozone and Aerosol Profiling

    NASA Technical Reports Server (NTRS)

    De Young, Russell; Carrion, William; Pliutau, Denis

    2014-01-01

    A compact mobile differential absorption lidar (DIAL) system has been developed at NASA Langley Research Center to provide ozone, aerosol and cloud atmospheric measurements in a mobile trailer for ground-based atmospheric ozone air quality campaigns. This lidar is integrated into the Tropospheric Ozone Lidar Network (TOLNet) currently made up of four other ozone lidars across the country. The lidar system consists of a UV and green laser transmitter, a telescope and an optical signal receiver with associated Licel photon counting and analog channels. The laser transmitter consist of a Q-switched Nd:YLF inter-cavity doubled laser pumping a Ce:LiCAF tunable UV laser with all the associated power and lidar control support units on a single system rack. The system has been configured to enable mobile operation from a trailer and was deployed to Denver, CO July 15-August 15, 2014 supporting the DISCOVER-AQ campaign. Ozone curtain plots and the resulting science are presented.

  14. Vertical aerosol structure of Neptune - Constraints from center-to-limb profiles

    NASA Astrophysics Data System (ADS)

    Hammel, H. B.; Baines, K. H.; Bergstralh, J. T.

    1989-08-01

    New center-to-limb (CTL) equatorial region profiles of Neptune have been extracted from spatially well-resolved images. The 8900-A CTL profile entails the presence of material above the 5-mbar level whose optical depth is less than 0.5. CH4-band data admit of thin scattering hazes in the 0.4-1.5 bar pressure level, although optical depths must be lower than 0.05; so thin a haze falls short of the reflected flux at 6340 A, thereby implying the presence of another scattering layer deeper than 1.5 bars. A good fit to the observed reflectivity is obtained by a bright cloud layer with an optical depth of 3.0.

  15. Assessment of the CALIPSO Lidar 532 nm Attenuated Backscatter Calibration Using the NASA LaRC Airborne High Spectral Resolution Lidar

    NASA Technical Reports Server (NTRS)

    Rogers, Raymond R.; Hostetler, Chris A.; Hair, Johnathan W.; Ferrare, Richard A.; Liu, Zhaoyan; Obland, Michael D.; Harper, David B.; Cook, Anthony L.; Powell, Kathleen A.; Vaughan, Mark A.; Winker, David M.

    2011-01-01

    The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument on the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) spacecraft has provided global, high-resolution vertical profiles of aerosols and clouds since it became operational on 13 June 2006. On 14 June 2006, the NASA Langley Research Center (LaRC) High Spectral Resolution Lidar (HSRL) was deployed aboard the NASA Langley B-200 aircraft for the first of a series of 86 underflights of the CALIPSO satellite to provide validation measurements for the CALIOP data products. To better assess the range of conditions under which CALIOP data products are produced, these validation flights were conducted under both daytime and nighttime lighting conditions, in multiple seasons, and over a large range of latitudes and aerosol and cloud conditions. This paper presents a quantitative assessment of the CALIOP 532 nm calibration (through the 532 nm total attenuated backscatter) using an internally calibrated airborne HSRL underflight data and is the most extensive study of CALIOP 532 nm calibration. Results show that average HSRL and CALIOP 532 nm total attenuated backscatter agree on average within 2.7% +/- 2.1% (CALIOP lower) at night and within 2.9 % +/- 3.9% (CALIOP lower) during the day., demonstrating the accuracy of the CALIOP 532 nm calibration algorithms. Additionally, comparisons with HSRL show consistency of the CALIOP calibration before and after the laser switch in 2009 as well as improvements in the daytime version 3 calibration scheme compared with the version 2 calibration scheme. Potential systematic uncertainties in the methodology relevant to validating satellite lidar measurements with an airborne lidar system are discussed and found to be less than 3.7% for this validation effort with HSRL. Results from this study are also compared to those from prior assessments of CALIOP calibration and attenuated backscatter.

  16. Observations of Stratospheric Aerosols over Sondrestrom, Greenland Injected by Russia's Sarychev Peak Volcano

    NASA Astrophysics Data System (ADS)

    Neely, R. R.; Thayer, J. P.; Hayman, M.; Barnes, J. E.; O'Neill, M.

    2009-12-01

    Volcanic stratospheric aerosols affect global climate by influencing the radiative budget and chemistry of the lower stratosphere. Presently the stratospheric aerosol levels are in a background state. This provides the opportunity for studies of stratospheric injections by small volcanic eruptions. A thin stratospheric aerosol layer was identified during the month of July, 2009 using the Arctic Lidar Technology (ARCLITE) System operated at Sondrestrom. Trajectory analysis points to the source of the aerosols being the Sarychev Peak volcano in the Russian Kuril Islands. Latitudinal observations of the layer were made by the NOAA/Earth System Research Laboratory/Global Monitoring Division’s (GMD) stratospheric lidar network (Boulder,CO; Mauna Loa, HI; and Pago Pago, American Samoa). These observations show a significant increase in aerosol backscatter levels compared to the low background levels observed prior the eruption. Profiles derived from the from the ARCLITE observations include depolarization, backscatter and temperature which allow for a characterization of the layer on a daily basis. The ARCLITE observations also provide a time series of measurements showing the evolution of the aerosol layer over the month after the injection within the context of the less frequent profiles provided by the global GMD network. From the optical qualities observed, the exact nature of the aerosols and their role in the radiative budget and stratospheric chemistry are elucidated. These types of observations are unique to ground based lidar systems like ARCLITE due to the optically thin qualities of the layer which prevent detection in the visible band by nadir looking satellites. The long-term effect of this injection of sulfur dioxide into the stratosphere may influence the formation of type 1b polar stratospheric clouds during the coming winter.

  17. Estimating Mixing Heights Using Microwave Temperature Profiler

    NASA Technical Reports Server (NTRS)

    Nielson-Gammon, John; Powell, Christina; Mahoney, Michael; Angevine, Wayne

    2008-01-01

    A paper describes the Microwave Temperature Profiler (MTP) for making measurements of the planetary boundary layer thermal structure data necessary for air quality forecasting as the Mixing Layer (ML) height determines the volume in which daytime pollution is primarily concentrated. This is the first time that an airborne temperature profiler has been used to measure the mixing layer height. Normally, this is done using a radar wind profiler, which is both noisy and large. The MTP was deployed during the Texas 2000 Air Quality Study (TexAQS-2000). An objective technique was developed and tested for estimating the ML height from the MTP vertical temperature profiles. In order to calibrate the technique and evaluate the usefulness of this approach, estimates from a variety of measurements during the TexAQS-2000 were compared. Estimates of ML height were used from radiosondes, radar wind profilers, an aerosol backscatter lidar, and in-situ aircraft measurements in addition to those from the MTP.

  18. Identification of aerosol composition from multi-wavelength lidar measurements

    NASA Technical Reports Server (NTRS)

    Wood, S. A.

    1984-01-01

    This paper seeks to develop the potential of lidar for the identification of the chemical composition of atmospheric aerosols. Available numerical computations suggest that aerosols can be identified by the wavelength dependence of aerosol optical properties. Since lidar can derive the volume backscatter coefficient as a function of wavelength, a multi-wavelength lidar system may be able to provide valuable information on the composition of aerosols. This research theoretically investigates the volume backscatter coefficients for the aerosol classes, sea-salts, and sulfates, as a function of wavelength. The results show that these aerosol compositions can be characterized and identified by their backscatter wavelength dependence. A method to utilize multi-wavelength lidar measurements to discriminate between compositionally different thin aerosol layers is discussed.

  19. Aerosol/Cloud Measurements Using Coherent Wind Doppler Lidars

    NASA Astrophysics Data System (ADS)

    Royer, Philippe; Boquet, Matthieu; Cariou, Jean-Pierre; Sauvage, Laurent; Parmentier, Rémy

    2016-06-01

    The accurate localization and characterization of aerosol and cloud layers is crucial for climate studies (aerosol indirect effect), meteorology (Planetary Boundary Layer PBL height), site monitoring (industrial emissions, mining,…) and natural hazards (thunderstorms, volcanic eruptions). LEOSPHERE has recently developed aerosol/cloud detection and characterization on WINDCUBE long range Coherent Wind Doppler Lidars (CWDL). These new features combine wind and backscatter intensity informations (Carrier-to-Noise Ratio CNR) in order to detect (aerosol/cloud base and top, PBL height) and to characterize atmospheric structures (attenuated backscatter, depolarization ratio). For each aerosol/cloud functionality the method is described, limitations are discussed and examples are given to illustrate the performances.

  20. The depolarization - attenuated backscatter relation: CALIPSO lidar measurements vs. theory.

    PubMed

    Hu, Yongxiang; Vaughan, Mark; Liu, Zhaoyan; Lin, Bing; Yang, Ping; Flittner, David; Hunt, Bill; Kuehn, Ralph; Huang, Jiangping; Wu, Dong; Rodier, Sharon; Powell, Kathy; Trepte, Charles; Winker, David

    2007-04-30

    Using measurements obtained by the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite, relationships between layer-integrated depolarization ratio (delta) and layer-integrated attenuated backscatter (gamma) are established for moderately thick clouds of both ice and water. A new and simple form of the delta-gamma relation for spherical particles, developed from Monte Carlo simulations and suitable for both water clouds and spherical aerosol particles, is found to agree well with the observations. A high-backscatter, low-depolarization delta-gamma relationship observed for some ice clouds is shown to result primarily from horizontally oriented plates and implies a preferential lidar ratio - depolarization ratio relation in nature for ice cloud particles containing plates.

  1. Micropulse lidar observations of tropospheric aerosols over northeastern South Africa during the ARREX and SAFARI 2000 dry season experiments

    NASA Astrophysics Data System (ADS)

    Campbell, James R.; Welton, Ellsworth J.; Spinhirne, James D.; Ji, Qiang; Tsay, Si-Chee; Piketh, Stuart J.; Barenbrug, Marguerite; Holben, Brent N.

    2003-07-01

    During the Aerosol Recirculation and Rainfall Experiment (ARREX 1999) and Southern African Regional Science Initiative (SAFARI 2000) dry season experiments, a micropulse lidar (523 nm) instrument was operated at the Skukuza Airport in northeastern South Africa. The lidar was colocated with a diverse array of passive radiometric equipment. For SAFARI 2000, a daytime time series of layer mean aerosol optical properties, including layer mean extinction-to-backscatter ratios and vertical extinction cross-section profiles are derived from the synthesis of the lidar data and aerosol optical depths from available AERONET Sun photometer data. Combined with derived spectral Angstrom exponents, normalized broadband flux measurements, and calculated air mass back-trajectories, the temporal evolution of the surface aerosol layer optical properties is analyzed for climatological trends. For dense biomass smoke events the extinction-to-backscatter ratio is between 50 and 90 sr, and corresponding spectral Angstrom exponent values are between 1.50 and 2.00. Observations of an advecting smoke event during SAFARI 2000 are shown. The smoke was embedded within two distinct stratified thermodynamic layers causing the particulate mass to advect over the instrument array in an incoherent manner on the afternoon of 1 September 2000. Significant surface broadband flux forcing of over -50 W/m2 was measured in this event. The evolution of the vertical aerosol extinction profile is profiled using the lidar data. Finally, observations of persistent elevated aerosol layers during ARREX 1999 are presented and discussed. Back-trajectory analyses combined with lidar and Sun photometer measurements indicate the likelihood for these aerosols being the result of long-range particulate transport from the southern and central South America.

  2. Demonstration of Aerosol Property Profiling by Multiwavelength Lidar Under Varying Relative Humidity Conditions

    NASA Technical Reports Server (NTRS)

    Veselovskii, I.; Whiteman, D. N.; Kolgotin, A.; Andrews, E.; Korenskii, M.

    2009-01-01

    During the months of July-August 2007 NASA conducted a research campaign called the Tropical Composition, Clouds and Climate Coupling (TC4) experiment. Vertical profiles of ozone were measured daily using an instrument known as an ozonesonde, which is attached to a weather balloon and launch to altitudes in excess of 30 km. These ozone profiles were measured over coastal Las Tablas, Panama (7.8N, 80W) and several times per week at Alajuela, Costa Rica (ION, 84W). Meteorological systems in the form of waves, detected most prominently in 100-300 in thick ozone layer in the tropical tropopause layer, occurred in 50% (Las Tablas) and 40% (Alajuela) of the soundings. These layers, associated with vertical displacements and classified as gravity waves ("GW," possibly Kelvin waves), occur with similar stricture and frequency over the Paramaribo (5.8N, 55W) and San Cristobal (0.925, 90W) sites of the Southern Hemisphere Additional Ozonesondes (SHADOZ) network. The gravity wave labeled layers in individual soundings correspond to cloud outflow as indicated by the tracers measured from the NASA DC-8 and other aircraft data, confirming convective initiation of equatorial waves. Layers representing quasi-horizontal displacements, referred to as Rossby waves, are robust features in soundings from 23 July to 5 August. The features associated with Rossby waves correspond to extra-tropical influence, possibly stratospheric, and sometimes to pollution transport. Comparison of Las Tablas and Alajuela ozone budgets with 1999-2007 Paramaribo and San Cristobal soundings shows that TC4 is typical of climatology for the equatorial Americas. Overall during TC4, convection and associated meteorological waves appear to dominate ozone transport in the tropical tropopause layer.

  3. Quantifying Wintertime Aerosol Nitrate Formation Pathways and Their Vertical Profiles in the Great Lakes Region of North America by CMAQ Process Analysis and Hourly Observations

    NASA Astrophysics Data System (ADS)

    Kim, Y.; Spak, S.; Carmichael, G. R.; Riemer, N. S.; Baek, J.; Fontaine, A.; Janssen, M.; Kenski, D. M.

    2012-12-01

    In order to better understand wintertime episodes of elevated fine particle (PM2.5) in the Great Lakes region, a modeling analysis using the CMAQ air quality model was conducted for January-March 2009, a period where special surface based observations were conducted at a pair of urban and rural sites in Wisconsin. The episodes are found to be regional and are characterized by low wind speeds, near-freezing temperatures, and elevated levels of ammonium nitrate. Integrated process rate (IPR) analysis and integrated reaction rate analysis (IRR) in 12 km regional simulations with the Community Multiscale Air Quality model (CMAQ) are employed to quantify contributions to nitrate formation from all simulated processes, most importantly local chemical production and transport. Substantial vertical profiles are found for nitric acid, nitrate, and N2O5. The maximum concentrations of aerosol nitrate occur at the surface and decrease with altitude. Nitric acid is produced most efficiently 50-200m above the surface at night. Surface concentrations of aerosol nitrate are maintained by downward transport via vertical diffusion. Aerosol nitrate is predominantly removed by dry deposition. The aerosol production rate is significantly higher during episodes, and both daytime and nighttime (N2O5) chemical pathways are important contributors to elevated concentrations. Near the surface at Milwaukee, the daytime formation pathway for nitric acid is larger than the nighttime pathways, while in rural areas, the relative magnitudes are reversed. Across the region, the importance of the nighttime pathway increases with altitude. A spatial analysis highlights regional variability at the surface layer and ~90m above surface for the period February 4 thru February 10, which includes two PM2.5 episodes. The net aerosol chemistry process rates and concentrations show the evolution of regional PM build-up of aerosol nitrate and nitric acid.

  4. Spectra of particulate backscattering in natural waters.

    PubMed

    Gordon, Howard R; Lewis, Marlon R; McLean, Scott D; Twardowski, Michael S; Freeman, Scott A; Voss, Kenneth J; Boynton, G Chris

    2009-08-31

    Hyperspectral profiles of downwelling irradiance and upwelling radiance in natural waters (oligotrophic and mesotrophic) are combined with inverse radiative transfer to obtain high resolution spectra of the absorption coefficient (a) and the backscattering coefficient (b(b)) of the water and its constituents. The absorption coefficient at the mesotrophic station clearly shows spectral absorption features attributable to several phytoplankton pigments (Chlorophyll a, b, c, and Carotenoids). The backscattering shows only weak spectral features and can be well represented by a power-law variation with wavelength (lambda): b(b) approximately lambda(-n), where n is a constant between 0.4 and 1.0. However, the weak spectral features in b(b)b suggest that it is depressed in spectral regions of strong particle absorption. The applicability of the present inverse radiative transfer algorithm, which omits the influence of Raman scattering, is limited to lambda < 490 nm in oligotrophic waters and lambda < 575 nm in mesotrophic waters. PMID:19724619

  5. Spectra of Particulate Backscattering in Natural Waters

    NASA Technical Reports Server (NTRS)

    Gordon, Howard, R.; Lewis, Marlon R.; McLean, Scott D.; Twardowski, Michael S.; Freeman, Scott A.; Voss, Kenneth J.; Boynton, Chris G.

    2009-01-01

    Hyperspectral profiles of downwelling irradiance and upwelling radiance in natural waters (oligotrophic and mesotrophic) are combined with inverse radiative transfer to obtain high resolution spectra of the absorption coefficient (a) and the backscattering coefficient (bb) of the water and its constituents. The absorption coefficient at the mesotrophic station clearly shows spectral absorption features attributable to several phytoplankton pigments (Chlorophyll a, b, c, and Carotenoids). The backscattering shows only weak spectral features and can be well represented by a power-law variation with wavelength (lambda): b(sub b) approx. Lambda(sup -n), where n is a constant between 0.4 and 1.0. However, the weak spectral features in b(sub b), suggest that it is depressed in spectral regions of strong particle absorption. The applicability of the present inverse radiative transfer algorithm, which omits the influence of Raman scattering, is limited to lambda < 490 nm in oligotrophic waters and lambda < 575 nm in mesotrophic waters.

  6. Quantitative retrieval of aerosol optical properties by means of ceilometers

    NASA Astrophysics Data System (ADS)

    Wiegner, Matthias; Gasteiger, Josef; Geiß, Alexander

    2016-04-01

    In the last few years extended networks of ceilometers have been established by several national weather services. Based on improvements of the hardware performance of these single-wavelength backscatter lidars and their 24/7 availability they are increasingly used to monitor mixing layer heights and to derive profiles of the particle backscatter profile. As a consequence they are used for a wide range of applications including the dispersion of volcanic ash plumes, validation of chemistry transport models and air quality studies. In this context the development of automated schemes to detect aerosol layers and to identify the mixing layer are essential, in particular as the latter is often used as a proxy for air quality. Of equal importance is the calibration of ceilometer signals as a pre-requisite to derive quantitative optical properties. Recently, it has been emphasized that the majority of ceilometers are influenced by water vapor absorption as they operate in the spectral range of 905 - 910 nm. If this effect is ignored, errors of the aerosol backscatter coefficient can be as large as 50%, depending on the atmospheric water vapor content and the emitted wavelength spectrum. As a consequence, any other derived quantity, e.g. the extinction coefficient or mass concentration, would suffer from a significant uncertainty in addition to the inherent errors of the inversion of the lidar equation itself. This can be crucial when ceilometer derived profiles shall be used to validate transport models. In this presentation, the methodology proposed by Wiegner and Gasteiger (2015) to correct for water vapor absorption is introduced and discussed.

  7. Measurements of Vertical Profiles of Turbulence, Temperature, Ozone, Aerosols, and BrO over Sea Ice and Tundra Snowpack during BROMEX

    NASA Astrophysics Data System (ADS)

    Shepson, P.; Caulton, D.; Cambaliza, M. L.; Dhaniyala, S.; Fuentes, J. D.; General, S.; Halfacre, J. W.; Nghiem, S. V.; Perez Perez, L.; Peterson, P. K.; Platt, U.; Pohler, D.; Pratt, K. A.; Simpson, W. R.; Stirm, B.; Walsh, S. J.; Zielcke, J.

    2012-12-01

    During the BROMEX field campaign of March 2012, we conducted measurements of boundary layer structure, ozone, BrO and aerosol, from a light, twin-engine aircraft during eleven flights originating from Barrow, AK. Flights were conducted over the sea ice in the Beaufort and Chukchi Seas, and over the tundra from Barrow to the Brooks Range, with vertical profiles covering altitudes from the surface to 3.5km in the free troposphere. Flights over the course of one month allowed a variety of sea ice conditions, including open water, nilas, first year sea ice, and frost flowers, to be examined over the Chukchi Sea. Atmospheric turbulence was measured using a calibrated turbulence probe, which will enable characterization of both the structure and turbulence of the Arctic boundary layer. Ozone was measured using a 2B UV absorption instrument. A GRIMM optical particle counter was used to measure 0.25-4 μm sized aerosol particles. The MAX-DOAS instrument enabled measurements of BrO vertical profiles. The aircraft measurements can be used to connect the surface measurements of ozone and BrO from the "Icelander" buoys, and the surface sites at Barrow, with those measured on the aircraft. Here we will discuss the spatial variability/coherence in these data. A major question that will be addressed using these data is the extent to which bromine is activated through reactions at the snowpack/ice surface versus the surface of aerosols. Here we will present a preliminary analysis of the relationships between snow/ice surface types, aerosol size-resolved number concentrations, and the vertical profiles of ozone and BrO.

  8. Preliminary results of the Vega 1 and Vega 2 optical investigation of aerosol in the atmosphere of Venus at 30-60 KM

    NASA Technical Reports Server (NTRS)

    Moshkin, B. Y.; Moroz, V. I.; Gnedykh, V. I.; Grigoryev, A. V.

    1986-01-01

    Aerosol concentration profiles were measured by an aerosol spectrometer above the landing sites of the Vega 1 and Vega 2 landers. Approximately the same altitude zones were found as in previous experiments: a three-layered basic cloud cover, an intermediate zone and subcloud haze. There were significant quantitative differences in the concentrations of particles, however, and especially in the spectra of their dimensions. Nightglow was found in the troposphere of Venus at a wavelength of about 1 micron. The backscatter coefficient and the extinction coefficient change very little between 32 and 63 km. Large numbers of submicron particles apparently exist in the atmosphere above the landing sites.

  9. Aerosol pattern correlation techniques of wind measurement

    NASA Technical Reports Server (NTRS)

    Eloranta, Edwin W.

    1985-01-01

    This paper reviews the current status of lidar image correlation techniques of remote wind measurement. It also examines the potential use of satellite borne lidar global wind measurements using this approach. Lidar systems can easily detect spatial variations in the volume scattering cross section of naturally occurring aerosols. Lidar derived RHI, PPI and range-time displays of aerosol backscatter have been extensively employed in the study of atmospheric structure. Descriptions of this type of data can be obtained in many references including Kunkel et al. (1977), Kunkel et al. (1980), Boers et al. (1984), Uthe et al. (1980), Melfi et al. (1985) and Browell et al. (1983). It is likely that the first space-borne lidars for atmospheric studies will observe aerosol backscatter to measure parameters such as boundary layer depth and cloud height. This paper examines the potential application of these relatively simple aerosol backscatter lidars to global wind measurements.

  10. Evaluation of Daytime Measurements of Aerosols and Water Vapor made by an Operational Raman Lidar over the Southern Great Plains

    NASA Technical Reports Server (NTRS)

    Ferrare, Richard; Turner, David; Clayton, Marian; Schmid, Beat; Covert, David; Elleman, Robert; Orgren, John; Andrews, Elisabeth; Goldsmith, John E. M.; Jonsson, Hafidi

    2006-01-01

    Raman lidar water vapor and aerosol extinction profiles acquired during the daytime over the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site in northern Oklahoma (36.606 N, 97.50 W, 315 m) are evaluated using profiles measured by in situ and remote sensing instruments deployed during the May 2003 Aerosol Intensive Operations Period (IOP). The automated algorithms used to derive these profiles from the Raman lidar data were first modified to reduce the adverse effects associated with a general loss of sensitivity of the Raman lidar since early 2002. The Raman lidar water vapor measurements, which are calibrated to match precipitable water vapor (PWV) derived from coincident microwave radiometer (MWR) measurements were, on average, 5-10% (0.3-0.6 g/m(exp 3) higher than the other measurements. Some of this difference is due to out-of-date line parameters that were subsequently updated in the MWR PWV retrievals. The Raman lidar aerosol extinction measurements were, on average, about 0.03 km(exp -1) higher than aerosol measurements derived from airborne Sun photometer measurements of aerosol optical thickness and in situ measurements of aerosol scattering and absorption. This bias, which was about 50% of the mean aerosol extinction measured during this IOP, decreased to about 10% when aerosol extinction comparisons were restricted to aerosol extinction values larger than 0.15 km(exp -1). The lidar measurements of the aerosol extinction/backscatter ratio and airborne Sun photometer measurements of the aerosol optical thickness were used along with in situ measurements of the aerosol size distribution to retrieve estimates of the aerosol single scattering albedo (omega(sub o)) and the effective complex refractive index. Retrieved values of omega(sub o) ranged from (0.91-0.98) and were in generally good agreement with omega(sub o) derived from airborne in situ measurements of scattering and absorption. Elevated aerosol

  11. Atmospheric aerosol characterization combining multi-wavelength Raman lidar and MAX-DOAS measurements in Gwanjgu

    NASA Astrophysics Data System (ADS)

    Chong, Jihyo; Shin, Dong Ho; Kim, Kwang Chul; Lee, Kwon-Ho; Shin, Sungkyun; Noh, Young M.; Müller, Detlef; Kim, Young J.

    2011-11-01

    Integrated approach has been adopted at the ADvanced Environmental Research Center (ADEMRC), Gwangju Institute of Science and Technology (GIST), Korea for effective monitoring of atmospheric aerosol. Various active and passive optical remote sensing techniques such as multi-wavelength (3β+2α+1δ) Raman LIDAR, sun-photometry, MAX-DOAS, and satellite retrieval have been utilized. This integrated monitoring system approach combined with in-situ surface measurement is to allow better characterization of physical and optical properties of atmospheric aerosol. Information on the vertical distribution and microphysical properties of atmospheric aerosol is important for understanding its transport characteristics as well as radiative effect. The GIST multi-wavelength (3β + 2α+1δ) Raman lidar system can measure vertical profiles of optical properties of atmospheric aerosols such as extinction coefficients at 355 and 532nm, particle backscatter coefficients at 355, 532 and 1064 nm, and depolarization ratio at 532nm. The incomplete overlap between the telescope field-of-view and beam divergence of the transmitting laser significantly affects lidar measurement, resulting in higher uncertainty near the surface where atmospheric aerosols of interest are concentrated. Differential Optical Absorption Spectroscopy (DOAS) technique is applied as a complementary tool for the detection of atmospheric aerosols near the surface. The passive Multi-Axis DOAS (MAX-DOAS) technique uses scattered sunlight as a light source from several viewing directions. Recently developed aerosol retrieval algorithm based on O4 slant column densities (SCDs) measured at UV and visible wavelengths has been utilized to derive aerosol information (e.g., aerosol optical depth (AOD) and aerosol extinction coefficients (AECs)) in the lower troposphere. The aerosol extinction coefficient at 356 nm was retrieved for the 0-1 and 1-2 km layers based on the MAX-DOAS measurements using the retrieval algorithm

  12. Initial characterization of micafungin pulmonary delivery via two different nebulizers and multivariate data analysis of aerosol mass distribution profiles.

    PubMed

    Shi, Shuai; Ashley, Elizabeth S Dodds; Alexander, Barbara D; Hickey, Anthony J

    2009-01-01

    Pharmaceutical aerosols have been targeted to the lungs for the treatment of asthma and pulmonary infectious diseases successfully. Micafungin (Astellas Pharma US, Deerfield, IL, USA) has been shown to be an effective antifungal agent when administrated intravenously. Pulmonary delivery of micafungin has not previously been reported. In the present pilot study, we characterize the performance of two nebulizers and their potential for delivering micafungin to the lungs as well as the use of multivariate data analysis for mass distribution profile comparison. The concentration of micafungin sodium increased by 21% when delivered by the Acorn II nebulizer and by 20% when delivered by the LC Plus nebulizer, respectively, from the first to the second sampling period. The Acorn II nebulizer delivered a fine particle fraction FPF(5.8) (%<5.8 microm) of 92.5 +/- 0.8 and FPF(3.3) (%<3.3 microm) of 82.3 +/- 2.1 during the first sampling period. For the LC Plus nebulizer, FPF(5.8) was 92.3 +/- 0.1 and FPF(3.3) was 67.0 +/- 0.7 during the first sampling period. The mass median aerodynamic diameter (MMAD) increased from 1.67 +/- 0.05 to 1.77 +/- 0.04 mum (Acorn II nebulizer) and from 2.09 +/- 0.01 to 2.20 +/- 0.01 microm (Pari LC Plus nebulizer) from the first to the second sampling periods. These changes in MMAD were statistically significant by paired t test. Multivariate data analysis showed that this could be explained systematically by greater drug deposition on stages with larger cutoff sizes and reduced drug deposition on stages with smaller cutoff sizes rather than multimodal deposition or other anomalies in size distribution.

  13. Aerosol vertical distribution, optical properties and transport over Corsica (western Mediterranean)

    NASA Astrophysics Data System (ADS)

    Léon, J.-F.; Augustin, P.; Mallet, M.; Bourrianne, T.; Pont, V.; Dulac, F.; Fourmentin, M.; Lambert, D.; Sauvage, B.

    2015-03-01

    This paper presents the aerosol vertical distribution observed in the western Mediterranean between February and April 2011 and between February 2012 and August 2013. An elastic backscattering lidar was continuously operated at a coastal site in the northern part of Corsica Island (Cap Corse) for a total of more than 14 000 h of observations. The aerosol extinction coefficient retrieved from cloud-free lidar profiles are analyzed along with the SEVIRI satellite aerosol optical depth (AOD). The SEVIRI AOD was used to constrain the retrieval of the aerosol extinction profiles from the lidar range-corrected signal and to detect the presence of dust or pollution aerosols. The daily average AOD at 550 nm is 0.16 (±0.09) and ranges between 0.05 and 0.80. A seasonal cycle is observed with minima in winter and maxima in spring-summer. High AOD days (above 0.3 at 550 nm) represent less than 10% of the totality of daily observations and correspond to the large scale advection of desert dust from Northern Africa or pollution aerosols from Europe. The respective origin of the air masses is confirmed using FLEXPART simulations in the backward mode. Dust events are characterized by a large turbid layer between 2 and 5 km height while pollution events show a lower vertical development with a thick layer below 3 km in altitude. However low level dust transport is also reported during spring while aerosol pollution layer between 2 and 4 km height has been also observed. We report an effective lidar ratio at 355 nm for pollution aerosols 68 (±13) Sr while it is 63 (±18) Sr for dust. The daily mean AOD at 355 nm for dust events is 0.61 (±0.14) and 0.71 (±0.16) for pollution aerosols events.

  14. Aerosol chemistry in Beijing, China: Different pollution regimes and diurnal profiles

    NASA Astrophysics Data System (ADS)

    van Pinxteren, D.; Brüggemann, E.; Gnauk, T.; Iinuma, Y.; Müller, K.; Nowak, A.; Achtert, P.; Wiedensohler, A.; Herrmann, H.

    2009-04-01

    The rapid economic development during the last three decades in China has led to a severe decrease in air quality, especially in densely populated regions such as Beijing, Shanghai, and the Pearl River Delta. Although during last years a number of measures for air pollution control have been implemented especially in the capital Beijing, air pollution is still regarded to be one of the top environmental concerns in China during the next decade. To better characterize the processes leading to the frequently observed high concentrations of air pollutants on a regional scale, the international field campaign "Campaigns of Air Quality Research in Beijing 2006" (CAREBEIJING2006) was conducted in summer 2006. Organized by the Peking University, project partners from Japan, Korea, Hong Kong, Germany, and China studied the various aspects of gaseous and particulate air pollution in a megacity environment. In this contribution, we present chemical data of size-resolved particles, obtained by a 5-stage Berner impactor (0.05-10 μm) during 3 weeks at both an urban and a suburban site in the area of Beijing, China. The sampling time of the impactors was about 4-5 hours. This allowed for taking four size-resolved samples per day and obtaining rough diurnal profiles of particle components. The samples were analyzed for inorganic ions (Cl-, SO42-, NO3-, NH4+, K+, Ca2+, Na+, Mg2+), carbon sum parameters (OC, EC, WSOC), and a variety of organic compounds such as dicarboxylic acids, alkanes, PAHs and, for the first time in China, nitrooxy-organosulfates. On average, the observed PM10 mass concentrations were 133 μg m-3 and 112 μg m-3 at the urban and suburban site, respectively. In general, the observed concentrations of particulate pollutants were similarly high as reported from previous studies in the Beijing summer atmosphere. A back trajectory analysis allowed the classification of the samples into different meteorological categories with different air mass origins. A high

  15. Microphysical Properties of Aerosols Encountered During the 2012 TCAP Campaign Using the Research Scanning Polarimeter

    NASA Astrophysics Data System (ADS)

    Stamnes, S.; Ferrare, R. A.; Hostetler, C. A.; Burton, S. P.; Liu, X.; Cairns, B.

    2015-12-01

    The Two-Column Aerosol Project (TCAP) campaign was conducted during the summer of 2012, off the East coast of the United States by Cape Cod. The NASA GISS Research Scanning Polarimeter, a multi-angle, multi-spectral polarimeter measured the upwelling polarized radiances from a B200 aircraft over a period of several weeks and over a distance of several hundred kilometers. A new algorithm based on optimal estimation that can retrieve aerosol microphysical properties using highly accurate radiative transfer and Mie calculations is presented. First, results for synthetic simulated data are discussed. The algorithm is then applied to real data collected during TCAP to retrieve the aerosol microphysical state vector and corresponding uncertainty for the aerosols that were encountered. Simultaneous measurements were also made by the NASA Langley airborne High Spectral Resolution Lidar (HSRL2), which provided extinction and backscatter profiles. The RSP-retrieved microphysical properties are compared to the extinction and backscatter products, and to the HSRL2-retrieved microphysical products.

  16. Modeling LIDAR Detection of Biological Aerosols to Determine Optimum Implementation Strategy

    SciTech Connect

    Sheen, David M.; Aker, Pam M.

    2007-09-19

    This report summarizes work performed for a larger multi-laboratory project named the Background Interferent Measurement and Standards project. While originally tasked to develop algorithms to optimize biological warfare agent detection using UV fluorescence LIDAR, the current uncertainties in the reported fluorescence profiles and cross sections the development of any meaningful models. It was decided that a better approach would be to model the wavelength-dependent elastic backscattering from a number of ambient background aerosol types, and compare this with that generated from representative sporulated and vegetative bacterial systems. Calculations in this report show that a 266, 355, 532 and 1064 nm elastic backscatter LIDAR experiment will allow an operator to immediately recognize when sulfate, VOC-based or road dust (silicate) aerosols are approaching, independent of humidity changes. It will be more difficult to distinguish soot aerosols from biological aerosols, or vegetative bacteria from sporulated bacteria. In these latter cases, the elastic scattering data will most likely have to be combined with UV fluorescence data to enable a more robust categorization.

  17. Seasonal Variations In Titan’s Stratosphere Observed With Cassini/CIRS: Temperature, Trace Molecular Gas And Aerosol Mixing Ratio Profiles

    NASA Astrophysics Data System (ADS)

    Vinatier, Sandrine; Bézard, B.; Anderson, C.; Teanby, N.; de Kok, R.; Actherberg, R.; Coustenis, A.; CIRS Team

    2012-10-01

    Titan's northern spring equinox occurred in August 2009. General Circulation Models predict strong modifications of the global circulation in this period, with formation of two circulation cells instead of the pole-to-pole cell that occurred during northern winter. This winter single cell, which had its descending branch at the north pole, was at the origin of the enrichment of molecular abundances and high stratopause temperatures observed by Cassini/CIRS at high northern latitudes. The predicted dynamical seasonal variations after the equinox have strong impact on the spatial distributions of trace gas, temperature and aerosol abundances. We will present here an analysis of CIRS limb-geometry datasets acquired in 2010, 2011 and 2012 that we used to monitor the seasonal evolution of the vertical profiles of temperature, molecular (C2H2, C2H6, HCN, ...) and aerosol abundances.

  18. Effect of CALIPSO Cloud Aerosol Discrimination (CAD) Confidence Levels on Observations of Aerosol Properties near Clouds

    NASA Technical Reports Server (NTRS)

    Yang, Weidong; Marshak, Alexander; Varnai, Tamas; Liu, Zhaoyan

    2012-01-01

    CALIPSO aerosol backscatter enhancement in the transition zone between clouds and clear sky areas is revisited with particular attention to effects of data selection based on the confidence level of cloud-aerosol discrimination (CAD). The results show that backscatter behavior in the transition zone strongly depends on the CAD confidence level. Higher confidence level data has a flatter backscatter far away from clouds and a much sharper increase near clouds (within 4 km), thus a smaller transition zone. For high confidence level data it is shown that the overall backscatter enhancement is more pronounced for small clear-air segments and horizontally larger clouds. The results suggest that data selection based on CAD reduces the possible effects of cloud contamination when studying aerosol properties in the vicinity of clouds.

  19. Balloonborne meaurements of Pinatubo aerosol during 1991 and 1992 at 41[degrees] N: Verticle profiles, size distribution, and volatility

    SciTech Connect

    Deshler, T.; Johnson, B.J.; Rozier, W.R.

    1993-07-23

    The authors report balloon borne measurements of the aerosol loading above Laramie, Wyoming from June, 1991, following the eruption of the Mt Pinatubo volcano. Estimates place the stratospheric loading at 20 to 30 Mtons of SO[sub 2] from this eruption. The authors measure the densities of condensation nuclei, with r > 0.01[mu]m, and of optical aerosols, with r > 0.15[mu]m. Following an initial peaking, the mass loading, and total scattering surface areas were observed to peak roughly 180 days after the eruption. In most of 1992 the aerosol observations remained fairly homogeneous and constant. Volatility measurements indicated the aerosol was mainly a mixture of water and sulfuric acid.

  20. Aircraft vertical profiles of trace gas and aerosol pollution over the mid-Atlantic United States: Statistics and meteorological cluster analysis

    NASA Astrophysics Data System (ADS)

    Taubman, B. F.; Hains, J. C.; Thompson, A. M.; Marufu, L. T.; Doddridge, B. G.; Stehr, J. W.; Piety, C. A.; Dickerson, R. R.

    2006-05-01

    From 1997 to 2003, airborne measurements of O3, CO, SO2, and aerosol properties were made during summertime air pollution episodes over the mid-Atlantic United States (34.7-44.6°N, 68.4-81.6°W) as part of the Regional Atmospheric Measurement, Modeling, and Prediction Program (RAMMPP). Little diurnal variation was identified in the CO, SO2, and Ångström exponent profiles, although the Ångström exponent profiles decreased with altitude. Boundary layer O3 was greater in the afternoon, while lower free tropospheric O3 was invariant at ˜55 ppbv. The single scattering albedo increased from morning to afternoon (0.93 ± 0.01-0.94 ± 0.01); however, both profiles decreased with altitude. A cluster analysis of back trajectories in conjunction with the vertical profile data was used to identify source regions and characteristic transport patterns during summertime pollution episodes. When the greatest trajectory density lay over the northern Ohio River Valley, the result was large O3 values, large SO2/CO ratios, highly scattering particles, and large aerosol optical depths. Maximum trajectory density over the southern Ohio River Valley resulted in little pollution. The greatest afternoon O3 values occurred during periods of stagnation. North-northwesterly and northerly flow brought the least pollution overall. The contribution of regional transport to afternoon boundary layer O3 was quantified. When the greatest cluster trajectory density lay over the Ohio River Valley (˜59% of the profiles), transport accounted for 69-82% of the afternoon boundary layer O3. Under stagnant conditions (˜27% of the profiles), transport only accounted for 58% of the afternoon boundary layer O3. The results from this study provide a description of regional chemical and transport processes that will be valuable to investigators from the Baltimore, New York, and Pittsburgh EPA Supersites.

  1. Extinction-to-Backscatter Ratios of Saharan Dust Layers Derived from In-Situ Measurements and CALIPSO Overflights During NAMMA

    NASA Technical Reports Server (NTRS)

    Omar, Ali H.; Liu, Zhaoyan; Vaughan, Mark A.; Hu, Yongxiang; Ismail, Syed; Powell, Kathleen A.; Winker, David M.; Trepte, Charles R.; Anderson, Bruce E.

    2010-01-01

    We determine the aerosol extinction-to-backscatter (Sa) ratios of dust using airborne in-situ measurements of microphysical properties, and CALIPSO observations during the NASA African Monsoon Multidisciplinary Analyses (NAMMA). The NAMMA field experiment was conducted from Sal, Cape Verde during Aug-Sept 2006. Using CALIPSO measurements of the attenuated backscatter of lofted Saharan dust layers, we apply the transmittance technique to estimate dust Sa ratios at 532 nm and a 2-color method to determine the corresponding 1064 nm Sa. Using this method, we found dust Sa ratios of 39.8 plus or minus 1.4 sr and 51.8 plus or minus 3.6 sr at 532 nm and 1064 nm, respectively. Secondly, Sa ratios at both wavelengths is independently calculated using size distributions measured aboard the NASA DC-8 and estimates of Saharan dust complex refractive indices applied in a T-Matrix scheme. We found Sa ratios of 39.1 plus or minus 3.5 sr and 50.0 plus or minus 4 sr at 532 nm and 1064 nm, respectively, using the T-Matrix calculations applied to measured size spectra. Finally, in situ measurements of the total scattering (550 nm) and absorption coefficients (532 nm) are used to generate an extinction profile that is used to constrain the CALIPSO 532 nm extinction profile.

  2. A New Approach to Inverting and De-Noising Backscatter from Lidar Observations

    NASA Astrophysics Data System (ADS)

    Marais, Willem; Hen Hu, Yu; Holz, Robert; Eloranta, Edwin

    2016-06-01

    Atmospheric lidar observations provide a unique capability to directly observe the vertical profile of cloud and aerosol scattering properties and have proven to be an important capability for the atmospheric science community. For this reason NASA and ESA have put a major emphasis on developing both space and ground based lidar instruments. Measurement noise (solar background and detector noise) has proven to be a significant limitation and is typically reduced by temporal and vertical averaging. This approach has significant limitations as it results in significant reduction in the spatial information and can introduce biases due to the non-linear relationship between the signal and the retrieved scattering properties. This paper investigates a new approach to de-noising and retrieving cloud and aerosol backscatter properties from lidar observations that leverages a technique developed for medical imaging to de-blur and de-noise images; the accuracy is defined as the error between the true and inverted photon rates. Hence non-linear bias errors can be mitigated and spatial information can be preserved.

  3. Aerosol and Water Vapor Raman Lidar System at CEILAP, Buenos Aires, Argentina. Case Study: November 07, 2006.

    NASA Astrophysics Data System (ADS)

    Otero, Lidia Ana; Ristori, Pablo Roberto; Quel, Eduardo Jaime

    2008-04-01

    A multiwavelength backscatter LIDAR (Light Detection And Ranging) was developed and operates at Centro de Investigaciones en Láseres y Aplicaciones, CEILAP (CITEFA-CONICET), (34.5 S and 58.5 W) to study the atmospheric properties such as the aerosol optical parameters, the boundary layer evolution, and the water vapor vertical distribution. The emission system is based on a Nd:YAG laser emitting at the fundamental, second and third harmonic wavelengths. The reception unit was upgraded to collect the atmospheric elastic and nitrogen Raman backscatters from the second and third harmonic wavelength and the water vapor Raman backscatter from the third harmonic wavelength. The information from all these channels give us enough information to derive the vertical distribution of the total to molecular backscatter, the backscatter to extinction ratio (lidar ratio) and the Ångström coefficient. In addition, water vapor mixing ratio profile is also measured by using the Raman water vapor and nitrogen channels (408 and 387 nm).

  4. Retrieval of atmospheric particles optical properties by combining ground-based and spaceborne lidar elastic scattering profiles.

    PubMed

    Wang, Xuan; Frontoso, Maria Grazia; Pisani, Gianluca; Spinelli, Nicola

    2007-05-28

    A simple algorithm is derived to retrieve the aerosol backscattering and extinction vertical profiles from simultaneously detected ground and space elastic lidar signals, without any a priori hypothesis on aerosol particles properties. This technique can be applied at any wavelength whenever two "counter looking" lidars are available and the atmosphere can be considered horizontally homogeneous in a spatial scale of the order of the distance between the two lidar beams. To test the accuracy of the algorithm a numerical simulation has been performed. Moreover, it has been applied in a real case to level 1 products from CALIPSO. PMID:19546983

  5. A New Raman DIAL Technique for Measuring Stratospheric Ozone in the Presence of Volcanic Aerosols

    NASA Technical Reports Server (NTRS)

    Singh, Upendra N.; Mcgee, Thomas J.; Gross, Michael; Heaps, William S.; Ferrare, Richard

    1992-01-01

    This paper describes a new lidar scheme to measure stratospheric ozone in the presence of heavy volcanic aerosol loading. The eruptions of the Philippine volcano Pinatubo during June 1991 ejected large amounts of sulfur dioxide into the atmosphere to altitudes of at least 30 km. The resulting aerosols have severely affected the measurements of stratospheric ozone when using traditional Rayleigh differential absorption lidar (DIAL) technique, in which the scattering mechanism is almost entirely Rayleigh and which assumes a small amount or no aerosols. In order to extract an ozone profile in the regions below about 30 km where the Rayleigh lidar returns are contaminated by aerosol scattering from Mt. Pinatubo cloud, we have used a Raman lidar technique, where the scattering mechanism depends solely on molecular nitrogen. In this scheme there is no aerosol scattering component to the backscattered lidar return. Using this technique in conjunction with the Rayleigh DIAL measurement, the GSFC stratospheric ozone lidar has measured ozone profiles between 15 and 50 km during the recently held UARS correlative measurement campaign (February-March 1992) at JPL's Table Mountain Facility in California.

  6. 1064 nm rotational Raman lidar for particle extinction and lidar-ratio profiling: cirrus case study

    NASA Astrophysics Data System (ADS)

    Haarig, Moritz; Engelmann, Ronny; Ansmann, Albert; Veselovskii, Igor; Whiteman, David N.; Althausen, Dietrich

    2016-09-01

    For the first time, vertical profiles of the 1064 nm particle extinction coefficient obtained from Raman lidar observations at 1058 nm (nitrogen and oxygen rotational Raman backscatter) are presented. We applied the new technique in the framework of test measurements and performed several cirrus observations of particle backscatter and extinction coefficients, and corresponding extinction-to-backscatter ratios at the wavelengths of 355, 532, and 1064 nm. The cirrus backscatter coefficients were found to be equal for all three wavelengths keeping the retrieval uncertainties in mind. The multiple-scattering-corrected cirrus extinction coefficients at 355 nm were on average about 20-30 % lower than the ones for 532 and 1064 nm. The cirrus-mean extinction-to-backscatter ratio (lidar ratio) was 31 ± 5 sr (355 nm), 36 ± 5 sr (532 nm), and 38 ± 5 sr (1064 nm) in this single study. We further discussed the requirements needed to obtain aerosol extinction profiles in the lower troposphere at 1064 nm with good accuracy (20 % relative uncertainty) and appropriate temporal and vertical resolution.

  7. Aerosol Layering Characterization Near the Gobi Desert by a Double Polarization Lidar System

    NASA Astrophysics Data System (ADS)

    Zhao, Y.; Boselli, A.; Sannino, A.; Song, C.; Spinelli, N.; Wang, X.

    2016-06-01

    In order to carry out 4-D (space and time) analysis of the atmospheric aerosol distribution and to make a characterization of their properties and time evolution, a transportable multi-wavelength, Elastic/Raman scanning lidar system with angular scanning capability has been realized. The system uses a diode pumped Nd:YAG laser source, specifically designed for this device, and a receiving systems able to detect elastic signals at 355, 532 and 1064 nm and Raman signals at 386, 407 and 607 nm. It also allows to perform aerosol depolarization measurements at both 355nm and 532nm. A first measurement campaign has been carried out in Dunhuang, North-West of China, in the region of the Gobi desert with the aims to study and characterize desert dust at source. Optical properties of aerosol layers developing in the atmosphere have been analyzed and lidar data are discussed in terms of profiles of aerosol backscatter coefficient at 355nm, 532nm, aerosol extinction coefficient at 355nm, aerosol depolarization ratio at 355nm and 532nm and water vapor mixing ratio. Depolarization ratio measured simultaneously at two wavelengths allowed also to study its dependence on the wavelength.

  8. Relationship between the fraction of backscattered light and the asymmetry parameter

    NASA Astrophysics Data System (ADS)

    Horvath, Helmuth

    2015-04-01

    The fraction of backscattered light is defined as the ratio of the integral of the volume scattering function over the backward half solid angle divided by the integral of the volume scattering function over the full solid angle. It can be measured with an integrating nephelometer. On the other hand the asymmetry parameter is the integral over the full solid angle of the volume scattering function weighted with the cosine of the scattering angle divided by the integral of the volume scattering function. To determine the asymmetry parameter the measurement of the angular dependence of the volume scattering function is needed, which can be obtained e.g. with a polar nephelometer. The asymmetry parameter is an important input parameter for radiative transfer calculations in order to obtain information of effects of the atmospheric aerosol effects (climate, screening, visibility, and others). Unfortunately measurements of the asymmetry parameter of the atmospheric aerosol are scarce. It is obvious, that a relation between the asymmetry parameter and the backscattered fraction should exist: the smaller the backscattered fraction, the more asymmetric the scattering, thus the larger the asymmetry parameter. A large set of 6500 angular scattering data have been obtained at various locations of the world: Vienna (Austria), Kyoto (Japan), Granada (Spain) and Palencia (Spain). The aerosols in these locations were considerably different, ranging from continental, urban, maritime, to desert dust. The volume scattering function has been measured between 5° and 175° , the values for 0° to 5° and 175° to 180° have been obtained by extrapolation of the shape of the curve, thus the whole range of scattering angles was available for calculating the backscattered fraction and the asymmetry parameter of the aerosol. PIC A summary of all data is shown in figure 1. The majority of the data points suggest an unanimous relation between backscattering and asymmetry parameter. The

  9. Temperatures and aerosol opacities of the Mars atmosphere at aphelion: Validation and inter-comparison of limb sounding profiles from MRO/MCS and MGS/TES

    NASA Astrophysics Data System (ADS)

    Shirley, James H.; McConnochie, Timothy H.; Kass, David M.; Kleinböhl, Armin; Schofield, John T.; Heavens, Nicholas G.; McCleese, Daniel J.; Benson, Jennifer; Hinson, David P.; Bandfield, Joshua L.

    2015-05-01

    We exploit the relative stability and repeatability of the Mars atmosphere at aphelion for an inter-comparison of Mars Global Surveyor/Thermal Emission Spectrometer (MGS/TES) and Mars Reconnaissance Orbiter/Mars Climate Sounder (MRO/MCS) nighttime temperature profiles and aerosol opacity profiles in Mars years 25, 26, 29, 30, and 31. Cross-calibration of these datasets is important, as they together provide an extended climatology for this planetary atmosphere. As a standard of comparison we employ temperature profiles obtained by radio occultation methods during the MGS mission in Mars years 24, 25, and 26. We first compare both zonal mean TES limb sounding profiles and zonal mean MCS limb sounding profiles with zonal means of radio occultation temperature profiles for the same season (Ls = 70-80°) and latitudes (55-70°N). We employ a statistical z test for quantifying the degree of agreement of temperature profiles by pressure level. For pressures less than 610 Pa (altitudes > 3 km), the ensemble mean temperature difference between the radio occultation and TES limb sounding profiles found in these comparisons was 1.7 ± 0.7 K. The ensemble mean temperature difference between radio occultation and MCS profiles was 1.4 ± 1.0 K. These differences fall within the formal error estimates for both TES and MCS, validating the accuracy of the instruments and their respective retrieval algorithms. In the second phase of our investigation, we compare aphelion season zonal mean TES limb sounding temperature, water ice opacity, and dust opacity profiles with those obtained at the same latitudes in different years by MCS. The ensemble mean temperature difference found for three comparisons between TES and MCS zonal mean temperature profiles was 2.8 ± 2.1 K. MCS and TES temperatures between 610 Pa and 5 Pa from 55 to 70°N are largely in agreement (with differences < 2 K) when water ice aerosol opacities are comparable. Temperature differences increase when the opacities

  10. LASE Measurements of Water Vapor, Aerosol, and Cloud Distributions in Saharan Air Layers and Tropical Disturbances

    NASA Technical Reports Server (NTRS)

    Ismail, Syed; Ferrare, Richard A.; Browell, Edward V.; Kooi, Susan A.; Dunion, Jason P.; Heymsfield, Gerry; Notari, Anthony; Butler, Carolyn F.; Burton, Sharon; Fenn, Marta; Krishnamurti, T. N.; Chen, Gao; Anderson, Bruce

    2010-01-01

    LASE (Lidar Atmospheric Sensing Experiment) on-board the NASA DC-8 measured high resolution profiles of water vapor and aerosols, and cloud distributions in 14 flights over the eastern North Atlantic during the NAMMA (NASA African Monsoon Multidisciplinary Analyses) field experiment. These measurements were used to study African easterly waves (AEWs), tropical cyclones (TCs), and the Saharan Air Layer(s) (SAL). Interactions between the SAL and tropical air were observed during the early stages of the TC development. These LASE measurements represent the first simultaneous water vapor and aerosol lidar measurements to study the SAL and its impact on AEWs and TCs. Examples of profile measurements of aerosol scattering ratios, aerosol extinction coefficients, aerosol optical thickness, water vapor mixing ratios, RH, and temperature are presented to illustrate their characteristics in SAL, convection, and clear air regions. LASE data suggest that the SAL suppresses low-altitude convection at the convection-SAL interface region. Mid-level convection associated with the AEW and transport are likely responsible for high water vapor content observed in the southern regions of the SAL on August 20, 2008. This interaction is responsible for the transfer of about 7 x 10(exp 15) J latent heat energy within a day to the SAL. Measurements of lidar extinction-to-backscatter ratios in the range 36+/-5 to 45+/-5 are within the range of measurements from other lidar measurements of dust. LASE aerosol extinction and water vapor profiles are validated by comparison with onboard in situ aerosol measurements and GPS dropsonde water vapor soundings, respectively.

  11. Continental pollution in the western Mediterranean basin: vertical profiles of aerosol and trace gases measured over the sea during TRAQA 2012 and SAFMED 2013

    NASA Astrophysics Data System (ADS)

    Di Biagio, C.; Doppler, L.; Gaimoz, C.; Grand, N.; Ancellet, G.; Raut, J.-C.; Beekmann, M.; Borbon, A.; Sartelet, K.; Attié, J.-L.; Ravetta, F.; Formenti, P.

    2015-08-01

    In this study we present airborne observations of aerosol and trace gases obtained over the sea in the western Mediterranean basin during the TRAQA (TRansport and Air QuAlity) and SAFMED (Secondary Aerosol Formation in the MEDiterranean) campaigns in summer 2012 and 2013. A total of 23 vertical profiles were measured up to 5000 m above sea level over an extended area (40-45° N and 2° W-12° E) including the Gulf of Genoa, southern France, the Gulf of Lion, and the Spanish coast. During TRAQA and SAFMED the study area experienced a wide range of meteorological conditions which favoured pollution export from different sources located around the basin. Also, several events of dust outflows were measured during the campaigns. Observations from the present study show that continental pollution largely affects the western Mediterranean both close to coastal regions and in the open sea as far as ~ 250 km from the coastline. The measured aerosol scattering coefficient varies between ~ 20 and 120 Mm-1, while carbon monoxide (CO) and ozone (O3) mixing ratios are in the range of 60-165 and 30-85 ppbv, respectively. Pollution reaches 3000-4000 m in altitude and presents a very complex and highly stratified structure characterized by fresh and aged layers both in the boundary layer and in the free troposphere. Within pollution plumes the measured particle concentration in the Aitken (0.004-0.1 μm) and accumulation (0.1-1.0 μm) modes is between ~ 30 and 5000-6000 scm-3 (standard cm-3), which is comparable to the aerosol concentration measured in continental areas under pollution conditions. Additionally, our measurements indicate the presence of highly concentrated Aitken layers (10 000-15 000 scm-3) observed both close to the surface and in the free troposphere, possibly linked to the influence of new particle formation (NPF) episodes over the basin.

  12. Lidar beams in opposite directions for quality assessment of Cloud-Aerosol Lidar with Orthogonal Polarization spaceborne measurements.

    PubMed

    Cuesta, Juan; Flamant, Pierre H

    2010-04-20

    We present the "lidar beams in opposite directions" (LIBOD) technique and applications for quality assessment of spaceborne observations made by Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation satellite. LIBOD is applicable to standard total backscatter lidar because it does not require a priori knowledge of the particle extinction-to-backscatter ratio. In this paper, we present (i) an objective assessment of the lidar signal quality and representativity of correlative ground-based lidar and CALIOP measurements only using normalized range-corrected lidar signals and (ii) a numerical filtering and optimization technique for reducing the spurious oscillations induced by noisy signal differentiation as needed for retrieval of particle extinction coefficients and extinction-to-backscatter ratio profiles. Numerical simulations and Monte Carlo tests are conducted for assessing the performance of the LIBOD technique. The applications are illustrated with examples of actual correlative 532 nm lidar profiles from CALIOP and a ground-based lidar deployed in Tamanrasset in the heart of Sahara in 2006 and near Strasbourg, France, in 2007.

  13. Final Technical Report for Interagency Agreement No. DE-SC0005453 “Characterizing Aerosol Distributions, Types, and Optical and Microphysical Properties using the NASA Airborne High Spectral Resolution Lidar (HSRL) and the Research Scanning Polarimeter (RSP)”

    SciTech Connect

    Hostetler, Chris; Ferrare, Richard

    2015-01-13

    Measurements of the vertical profile of atmospheric aerosols and aerosol optical and microphysical characteristics are required to: 1) determine aerosol direct and indirect radiative forcing, 2) compute radiative flux and heating rate profiles, 3) assess model simulations of aerosol distributions and types, and 4) establish the ability of surface and space-based remote sensors to measure the indirect effect. Consequently the ASR program calls for a combination of remote sensing and in situ measurements to determine aerosol properties and aerosol influences on clouds and radiation. As part of our previous DOE ASP project, we deployed the NASA Langley airborne High Spectral Resolution Lidar (HSRL) on the NASA B200 King Air aircraft during major field experiments in 2006 (MILAGRO and MaxTEX), 2007 (CHAPS), 2009 (RACORO), and 2010 (CalNex and CARES). The HSRL provided measurements of aerosol extinction (532 nm), backscatter (532 and 1064 nm), and depolarization (532 and 1064 nm). These measurements were typically made in close temporal and spatial coincidence with measurements made from DOE-funded and other participating aircraft and ground sites. On the RACORO, CARES, and CalNEX missions, we also deployed the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). RSP provided intensity and degree of linear polarization over a broad spectral and angular range enabling column-average retrievals of aerosol optical and microphysical properties. Under this project, we analyzed observations and model results from RACORO, CARES, and CalNex and accomplished the following objectives. 1. Identified aerosol types, characterize the vertical distribution of the aerosol types, and partition aerosol optical depth by type, for CARES and CalNex using HSRL data as we have done for previous missions. 2. Investigated aerosol microphysical and macrophysical properties using the RSP. 3. Used the aerosol backscatter and extinction profiles measured by the HSRL

  14. Analysis of the Impact of Major Dust Events on the Aerosols Characteristics over Saudi Arabia

    NASA Astrophysics Data System (ADS)

    Farahat, Ashraf; El-Askary, Hesham; Al-Shaibani, Abdulaziz; Hariri, Mustafa M.

    2015-04-01

    The Kingdom of Saudi Arabia is a major source of atmospheric dust. Frequent dust storms blow up and significantly affect human activities, airports and citizens' health. Aerosols optical and physical characteristics are influenced by major dust storms outbreaks. In this, paper, ground based AERONET measurements are integrated with space-borne sensors, namely MODIS and CALIPSO to analyze aerosols' characteristics during March - May of 2009 where a massive dust storm blew up and caused a widespread heavy atmospheric dust load over Saudi Arabia and the same period during 2010, where less dust activities were reported. The MODIS Deep Blue AOD analysis showed similar aerosols pattern over the land, however a substantial variance in aerosol loading during March - May 2009 compared with the same period in 2010 was observed. The angstrom exponent analysis showed that the majority of aerosol measurements in 2009 and 2010 are dominated by coarse-mode particles with angstrom exponent < 0.5. Detailed analysis of aerosol optical properties shows significant influence of coarse mode particles in the enhanced aerosol loading in 2009. The volume depolarization rations (VDR) derived from CALIPSO backscattering measurements is used to find latitudinal profile of mean aerosol optical depth to indicate the type of particles and to discriminate spherical aerosols with non-spherical particles. Acknowledgement The authors would like to acknowledge the support provided by the King Abdel Aziz City for Science & Technology (KACST) for funding this work under grant No. (MT-32-76). The support provided by the Deanship of Research at King Fahd University of Petroleum & Minerals (KFUPM) is gratefully acknowledged.

  15. Comparison of Aerosol Single Scattering Albedos Derived by Diverse Techniques In Two North Atlantic Experiments

    NASA Technical Reports Server (NTRS)

    Russell, P. B.; Redemann, J.; Schmid, B.; Bergstrom, R. W.; Livingston, J. M.; McIntosh, D. M.; Ramirez, S. A.; Hartley, S.; Hobbs, P. V.; Quinn, P. K.

    2002-01-01

    Aerosol single scattering albedo omega (the ratio of scattering to extinction) is important in determining aerosol climatic effects, in explaining relationships between calculated and measured radiative fluxes, and in retrieving aerosol optical depths from satellite radiances. Recently, two experiments in the North Atlantic region, the Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) and the Second Aerosol Characterization Experiment (ACE-2), determined aerosol omega by a variety of techniques. The techniques included fitting of calculated to measured radiative fluxes; retrievals of omega from skylight radiances; best fits of complex refractive index to profiles of backscatter extinction, and size distribution; and in situ measurements of scattering and absorption at the surface and aloft. Both TARFOX and ACE-2 found a fairly wide range of values for omega at midvisable wavelengths approx. 550 nm, with omega(sub midvis) greater than or equal to 0.85 and less than or equal to 0.99 for the marine aerosol impacted by continental pollution. Frequency distributions of omega could usually be approximated by lognormals in omega(sub max) - omega, with some occurrence of bimodality, suggesting the influence of different aerosol sources or processing. In both TARFOX and ACE-2, closure tests between measured and calculated radiative fluxes yielded best-fit values of omega(sub midvis) 0.90 +/- 0.04 for the polluted boundary layer. Although these results have the virtue of describing the column aerosol unperturbed by sampling, they are subject to questions about representativeness and other uncertainties (e.g., thermal offsets, unknown gas absorption) The other techniques gave larger values for omega(sub midvis) for the polluted boundary layer, with a typical result of omega(sub midvis) = 0.95 +/- 0.04. Current uncertainties in omega are large in terms of climate effects More tests are needed of the consistency among different methods and of

  16. Distribution of sulphuric acid aerosols in the clouds and upper haze of Venus using Venus Express VAST and VeRa temperature profiles

    NASA Astrophysics Data System (ADS)

    Parkinson, Christopher D.; Gao, Peter; Schulte, Rick; Bougher, Stephen W.; Yung, Yuk L.; Bardeen, Charles G.; Wilquet, Valérie; Vandaele, Ann Carine; Mahieux, Arnaud; Tellmann, Silvia; Pätzold, Martin

    2015-08-01

    Observations from Pioneer Venus and from SPICAV/SOIR aboard Venus Express (VEx) have shown the upper haze (UH) of Venus to be highly spatially and temporally variable, and populated by multiple particle size modes. Previous models of this system (e.g., Gao et al., 2014. Icarus 231, 83-98), using a typical temperature profile representative of the atmosphere (viz., equatorial VIRA profile), did not investigate the effect of temperature on the UH particle distributions. We show that the inclusion of latitude-dependent temperature profiles for both the morning and evening terminators of Venus helps to explain how the atmospheric aerosol distributions vary spatially. In this work we use temperature profiles obtained by two instruments onboard VEx, VeRa and SPICAV/SOIR, to represent the latitudinal temperature dependence. We find that there are no significant differences between results for the morning and evening terminators at any latitude and that the cloud base moves downwards as the latitude increases due to decreasing temperatures. The UH is not affected much by varying the temperature profiles; however, the haze does show some periodic differences, and is slightly thicker at the poles than at the equator. We also find that the sulphuric acid "rain" seen in previous models may be restricted to the equatorial regions of Venus, such that the particle size distribution is relatively stable at higher latitudes and at the poles.

  17. Radiative Effects of Aerosols

    NASA Technical Reports Server (NTRS)

    Valero, Francisco P. J.

    1997-01-01

    During the Atlantic Stratocumulus Transition Experiment (ASTEX) in June 1992, two descents in cloud-free regions allowed comparison of the change in aerosol optical depth as determined by an onboard total-direct-diffuse radiometer (TDDR) to the change calculated from measured size resolved aerosol microphysics and chemistry. Both profiles included pollution haze layer from Europe but the second also included the effect of a Saharan dust layer above the haze. The separate contributions of supermicrometer (coarse) and submicrometer (fine) aerosol were determined and thermal analysis of the pollution haze indicated that the fine aerosol was composed primarily of a sulfate/water mixture with a refractory soot-like core.

  18. Thermoluminescent aerosol analysis

    NASA Technical Reports Server (NTRS)

    Rogowski, R. S.; Long, E. R., Jr. (Inventor)

    1977-01-01

    A method for detecting and measuring trace amounts of aerosols when reacted with ozone in a gaseous environment was examined. A sample aerosol was exposed to a fixed ozone concentration for a fixed period of time, and a fluorescer was added to the exposed sample. The sample was heated in a 30 C/minute linear temperature profile to 200 C. The trace peak was measured and recorded as a function of the test aerosol and the recorded thermoluminescence trace peak of the fluorescer is specific to the aerosol being tested.

  19. Characterizing Aerosol Distributions and Optical Properties Using the NASA Langley High Spectral Resolution Lidar

    SciTech Connect

    Hostetler, Chris; Ferrare, Richard

    2013-02-14

    The objective of this project was to provide vertically and horizontally resolved data on aerosol optical properties to assess and ultimately improve how models represent these aerosol properties and their impacts on atmospheric radiation. The approach was to deploy the NASA Langley Airborne High Spectral Resolution Lidar (HSRL) and other synergistic remote sensors on DOE Atmospheric Science Research (ASR) sponsored airborne field campaigns and synergistic field campaigns sponsored by other agencies to remotely measure aerosol backscattering, extinction, and optical thickness profiles. Synergistic sensors included a nadir-viewing digital camera for context imagery, and, later in the project, the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). The information from the remote sensing instruments was used to map the horizontal and vertical distribution of aerosol properties and type. The retrieved lidar parameters include profiles of aerosol extinction, backscatter, depolarization, and optical depth. Products produced in subsequent analyses included aerosol mixed layer height, aerosol type, and the partition of aerosol optical depth by type. The lidar products provided vertical context for in situ and remote sensing measurements from other airborne and ground-based platforms employed in the field campaigns and was used to assess the predictions of transport models. Also, the measurements provide a data base for future evaluation of techniques to combine active (lidar) and passive (polarimeter) measurements in advanced retrieval schemes to remotely characterize aerosol microphysical properties. The project was initiated as a 3-year project starting 1 January 2005. It was later awarded continuation funding for another 3 years (i.e., through 31 December 2010) followed by a 1-year no-cost extension (through 31 December 2011). This project supported logistical and flight costs of the NASA sensors on a dedicated aircraft, the subsequent

  20. Atmospheric aerosols: Their Optical Properties and Effects (supplement)

    NASA Technical Reports Server (NTRS)

    1976-01-01

    A digest of technical papers is presented. Topics include aerosol size distribution from spectral attenuation with scattering measurements; comparison of extinction and backscattering coefficients for measured and analytic stratospheric aerosol size distributions; using hybrid methods to solve problems in radiative transfer and in multiple scattering; blue moon phenomena; absorption refractive index of aerosols in the Denver pollution cloud; a two dimensional stratospheric model of the dispersion of aerosols from the Fuego volcanic eruption; the variation of the aerosol volume to light scattering coefficient; spectrophone in situ measurements of the absorption of visible light by aerosols; a reassessment of the Krakatoa volcanic turbidity, and multiple scattering in the sky radiance.

  1. Ultrasonic backscatter from cancellous bone: the apparent backscatter transfer function.

    PubMed

    Hoffmeister, Brent K; Mcpherson, Joseph A; Smathers, Morgan R; Spinolo, P Luke; Sellers, Mark E

    2015-12-01

    Ultrasonic backscatter techniques are being developed to detect changes in cancellous bone caused by osteoporosis. Many techniques are based on measurements of the apparent backscatter transfer function (ABTF), which represents the backscattered power from bone corrected for the frequency response of the measurement system. The ABTF is determined from a portion of the backscatter signal selected by an analysis gate of width τw delayed by an amount τd from the start of the signal. The goal of this study was to characterize the ABTF for a wide range of gate delays (1 μs ≤ τd ≤ 6 μs) and gate widths (1 μs ≤ τw ≤ 6 μs). Measurements were performed on 29 specimens of human cancellous bone in the frequency range 1.5 to 6.0 MHz using a broadband 5-MHz transducer. The ABTF was found to be an approximately linear function of frequency for most choices of τd and τw. Changes in τd and τw caused the frequency-averaged ABTF [quantified by apparent integrated backscatter (AIB)] and the frequency dependence of the ABTF [quantified by frequency slope of apparent backscatter (FSAB)] to change by as much as 24.6 dB and 6.7 dB/MHz, respectively. τd strongly influenced the measured values of AIB and FSAB and the correlation of AIB with bone density (-0.95 ≤ R ≤ +0.68). The correlation of FSAB with bone density was influenced less strongly by τd (-0.97 ≤ R ≤ -0.87). τw had a weaker influence than τd on the measured values of AIB and FSAB and the correlation of these parameters with bone density.

  2. Aerosol and cloud typing with an automated 24/7 aerosol lidar

    NASA Astrophysics Data System (ADS)

    Baars, Holger; Seifert, Patric; Wandinger, Ulla

    2015-04-01

    Modern sophisticated multi-wavelength Raman polarization lidars have the ability to measure autonomous and unattended in 24/7 mode. These aerosol lidars can deliver backscatter, extinction, and depolarization profiles of the atmosphere which can be used for a target categorization, i.e. the determination of different aerosol and cloud types. However, to derive the optical particle properties a calibration of the lidar signals in the free atmosphere, where only Rayleigh scattering occurs, is needed. This calibration is usually done manually case by case and thus prohibits automatic data analysis and particle typing. To overcome this limitation, the mobile EARLINET lidar PollyXT of TROPOS was deployed continuously without changes in the instrumental setup during two field campaigns in the framework of the German HD(CP)2 project to obtain temporally stable lidar signals. The temporal stability together with the high performance and good characterization of the lidar lead to the possibility of an absolute lidar calibration. The corresponding calibration constant was derived in two ways: first by using manually Raman and Klett retrievals for selected periods and second by using the aerosol optical depth (AOD) from co-located AERONET sun photometer measurements. The derived calibration constants show a high temporal stability and a good agreement between both methods and thus allowed the continuous calibration of the lidar and the retrieval of the attenuated backscatter coefficient at three wavelengths. In addition, the calibrated volume depolarization ratio, obtained following EARLINET recommendations, is continuously available. After correction for the molecular contribution, these four quantities were used for an aerosol and cloud typing in terms of particle size and shape. The final categorization leads to 11 categories, e.g. clean atmosphere, small spherical particles, large non-spherical particles, water droplets, ice crystals and corresponding mixtures. In this

  3. Aerosol cloud interaction: a multiplatform-scenario-based methodology

    NASA Astrophysics Data System (ADS)

    Landulfo, Eduardo; Lopes, Fabío. J. S.; Guerrero-Rascado, Juan Luis; Alados-Arboledas, Lucas

    2015-10-01

    Suspended atmospheric particles i.e. aerosol particles go through many chemical and physical processes and those interactions and transformations may cause particle change in size, structure and composition regulated by mechanisms, which are also present in clouds. These interactions play a great role in the radiation transfer in the atmosphere and are not completely understood as competing effects might occur which are known as indirect aerosol effects. Performing measurements and experiments in remote sensing to improve the knowledge of these processes are also a challenge. In face of that we propose a multi-platform approach based lidar, sun photometry and satellite observations which should be characterized under a scenario perspective in which given the cloud height, geometric and optical geometries in a diurnal/nocturnal basis will make possible to apply different analytical tools in each a set of product that specify the aerosol present in the vicinity of clouds, their optical and physical properties. These scenarios are meant to aid in tagging the expected products and help in creating a robust database to systematically study the aerosol-cloud interaction.In total we will present 6 scenarios: 3 under daylight conditions, 3 under at nighttime. Each scenario and their counterpart should be able to provide the cloud base/top height, aerosol backscattering profile and cloud optical/geometric thickness. In each instance we should count on a 5 wavelength Raman lidar system measurement, a collocated sun photometer and CALIPSO/MODIS observation from AQUA/TERRA platforms. To further improve the aerosol cloud interaction the Raman lidar system should have a water vapor channel or moreover a liquid water channel. In our study we will present a two-day case study to show the methodology feasibility and its potential application.

  4. Mediterranean aerosol typing by integrating three-wavelength lidar and sun photometer measurements.

    PubMed

    Perrone, M R; Burlizzi, P

    2016-07-01

    Backscatter lidar measurements at 355, 532, and 1064 nm combined with aerosol optical thicknesses (AOTs) from sun photometer measurements collocated in space and time were used to retrieve the vertical profiles of intensive and extensive aerosol parameters. Then, the vertical profiles of the Ångström coefficients for different wavelength pairs (Å(λ1, λ2, z)), the color ratio (CR(z)), the fine mode fraction (η(z)) at 532 nm, and the fine modal radius (R f (z)), which represent aerosol characteristic properties independent from the aerosol load, were used for typing the aerosol over the Central Mediterranean. The ability of the Ångström coefficients to identify the main aerosol types affecting the Central Mediterranean with the support of the backward trajectory analysis was first demonstrated. Three main aerosol types, which were designed as continental-polluted (CP), marine-polluted (MP), and desert-polluted (DP), were identified. We found that both the variability range and the vertical profile structure of the tested aerosol intensive parameters varied with the aerosol type. The variability range and the altitude dependence of the aerosol extinction coefficients at 355, 532, and 1064 nm, respectively, also varied with the identified aerosol types even if they are extensive aerosol parameters. DP, MP, and CP aerosols were characterized by the Å(532, 1064 nm) mean values ± 1 standard deviation equal to 0.5 ± 0.2, 1.1 ± 0.2, 1.6 ± 0.2, respectively. η(%) mean values ± 1SD were equal to 50 ± 10, 73 ± 7, and 86 ± 6 for DP, MP, and CP aerosols, respectively. The R f and CR mean values ± 1SD were equal to 0.16 ± 0.05 μm and 1.3 ± 0.3, respectively, for DP aerosols; to 0.12 ± 0.03 μm and 1.8 ± 0.4, respectively, for MP aerosols; and to 0.11 ± 0.02 μm and 1.7 ± 0.4, respectively, for CP aerosols. CP and DP aerosols were on average responsible for greater AOT and LR values, but

  5. Continental pollution in the Western Mediterranean Basin: vertical profiles of aerosol and trace gases measured over the sea during TRAQA 2012 and SAFMED 2013

    NASA Astrophysics Data System (ADS)

    Di Biagio, C.; Doppler, L.; Gaimoz, C.; Grand, N.; Ancellet, G.; Raut, J.-C.; Beekmann, M.; Borbon, A.; Sartelet, K.; Attié, J.-L.; Ravetta, F.; Formenti, P.

    2015-03-01

    In this study we present airborne observations of aerosol and trace gases obtained over the sea in the Western Mediterranean Basin during the TRAQA (TRansport and Air QuAlity) and SAFMED (Secondary Aerosol Formation in the MEDiterranean) campaigns in summers 2012 and 2013. A total of 23 vertical profiles were measured up to 5000 m a.s.l. over an extended area (40-45° N latitude and 2° W-12° E longitude) including the Gulf of Genoa, Southern France, the Gulf of Lion, and the Spanish coast. TRAQA and SAFMED successfully measured a wide range of meteorological conditions which favoured the pollution export from different sources located around the basin. Also, several events of dust outflows were measured during the campaigns. Observations from the present study indicate that continental pollution largely affects the Western Mediterranean both close to coastal regions and in the open sea as far as ~250 km from the coastline. Aerosol layers not specifically linked with Saharan dust outflows are distributed ubiquitously which indicates quite elevated levels of background pollution throughout the Western Basin. The measured aerosol scattering coefficient varies between ~20 and 120 M m-1, while carbon monoxide (CO) and ozone (O3) mixing ratios are in the range of 60-170 and 30-85 ppbv, respectively. Pollution reaches 3000-4000 m in altitude and presents a very complex and highly stratified structure characterized by fresh and aged layers both in the boundary layer and in the free troposphere. Within pollution plumes the measured particle concentration in the Aitken (0.004-0.1 μm) and accumulation (0.1-1.0 μm) modes is between ˜ 100 and 5000-6000 s cm-3 (standard cm-3), which is comparable to the aerosol concentration measured in continental urban areas. Additionally, our measurements indicate the presence of highly concentrated Aitken layers (10 000-15 000 s cm-3) observed both close to the surface and in the free troposphere, possibly linked to the influence of new

  6. Criteria of backscattering in chiral one-way photonic crystals

    NASA Astrophysics Data System (ADS)

    Cheng, Pi-Ju; Chang, Shu-Wei

    2016-03-01

    Optical isolators are important devices in photonic circuits. To reduce the unwanted reflection in a robust manner, several setups have been realized using nonreciprocal schemes. In this study, we show that the propagating modes in a strongly-guided chiral photonic crystal (no breaking of the reciprocity) are not backscattering-immune even though they are indeed insensitive to many types of scatters. Without the protection from the nonreciprocity, the backscattering occurs under certain circumstances. We present a perturbative method to calculate the backscattering of chiral photonic crystals in the presence of chiral/achiral scatters. The model is, essentially, a simplified analogy to the first-order Born approximation. Under reasonable assumptions based on the behaviors of chiral photonic modes, we obtained the expression of reflection coefficients which provides criteria for the prominent backscattering in such chiral structures. Numerical examinations using the finite-element method were also performed and the results agree well with the theoretical prediction. From both our theory and numerical calculations, we find that the amount of backscattering critically depends on the symmetry of scatter cross sections. Strong reflection takes place when the azimuthal Fourier components of scatter cross sections have an order l of 2. Chiral scatters without these Fourier components would not efficiently reflect the chiral photonic modes. In addition, for these chiral propagating modes, disturbances at the most significant parts of field profiles do not necessarily result in the most effective backscattering. The observation also reveals what types of scatters or defects should be avoided in one-way applications of chiral structures in order to minimize the backscattering.

  7. Moving Toward Continuous Satellite Monitoring of PM2.5 Using the GOES Aerosol/Smoke Product (GASP) and Aircraft Profiles

    NASA Astrophysics Data System (ADS)

    Stehr, J. W.; Kondragunta, S.; Anderson, D. C.; Arkinson, H.; Brent, L. C.; Goldberg, D.; He, H.; Liaskos, C.; Ring, A.; Dickerson, R. R.; Carpenter, S.; Ciren, P.; Xu, C.

    2012-12-01

    The NOAA Geostationary Operational Environmental Satellite (GOES) makes measurements of aerosol optical depth (AOD) every 30 minutes during daylight hours. Those measurements then feed the Automated Smoke Detection and Tracking algorithm that uses fire counts, trajectory modeling and pattern recognition to identify fire plumes, especially in the western U.S. Tying these satellite measurements to surface measurements of fine particles (PM2.5) would be a considerable benefit to the air quality community and to people who live in areas with elevated fine particle concentrations. Currently, these retrievals are useful in identifying areas of elevated PM2.5 concentrations and in forecasting PM2.5 by federal, state and local agencies, but are largely limited to qualitative measures of fine particle loading. Among other issues, layers of fine particles well above ground level, cloud contamination, and particle growth by addition of water in areas of high relative humidity are examples of barriers to a direct relationship between surface PM2.5 and satellite AOD. We have identified a path forward by using aircraft profiles to determine the vertical distribution of aerosol scattering in the atmosphere. In addition, long-term measurements of scattering and rapid measurements of PM2.5 at ground-based field sites have provided a relationship between scattering and mass. Simultaneous measurements of relative humidity and temperature allow one to calculate scattering the particles would have in a dry environment and relate that to fine particle mass measurements. A relationship between rapid scattering measurements and much slower PM2.5 mass measurements is then developed, which is used to tie rapid aircraft measurements of scattering to mass. In turn, aircraft profiles are then used to tie column measurements to those at the ground and to identify cases when satellite retrievals are likely to fail. The resulting algorithm should apply throughout much of the eastern U.S., so long

  8. 3D Backscatter Imaging System

    NASA Technical Reports Server (NTRS)

    Turner, D. Clark (Inventor); Whitaker, Ross (Inventor)

    2016-01-01

    Systems and methods for imaging an object using backscattered radiation are described. The imaging system comprises both a radiation source for irradiating an object that is rotationally movable about the object, and a detector for detecting backscattered radiation from the object that can be disposed on substantially the same side of the object as the source and which can be rotationally movable about the object. The detector can be separated into multiple detector segments with each segment having a single line of sight projection through the object and so detects radiation along that line of sight. Thus, each detector segment can isolate the desired component of the backscattered radiation. By moving independently of each other about the object, the source and detector can collect multiple images of the object at different angles of rotation and generate a three dimensional reconstruction of the object. Other embodiments are described.

  9. Atmospheric Temperature Profile Measurements Using Mobile High Spectral Resolution Lidar

    NASA Astrophysics Data System (ADS)

    Razenkov, Ilya I.; Eloranta, Edwin W.

    2016-06-01

    The High Spectral Resolution Lidar (HSRL) designed at the University of Wisconsin-Madison discriminates between Mie and Rayleigh backscattering [1]. It exploits the Doppler effect caused by thermal motion of molecules, which broadens the spectrum of the transmitted laser light. That allows for absolute calibration of the lidar and measurements of the aerosol volume backscatter coefficient. Two iodine absorption filters with different absorption line widths (a regular iodine vapor filter and Argon buffered iodine filter) allow for atmospheric temperature profile measurements. The sensitivity of the measured signal-to-air temperature ratio is around 0.14%/K. The instrument uses a shared telescope transmitter-receiver design and operates in eyesafe mode (the product of laser average power and telescope aperture equals 0.1 Wm2 at 532 nm).

  10. Properties of Sarychev sulphate aerosols over the Arctic

    NASA Astrophysics Data System (ADS)

    O'Neill, N. T.; Perro, C.; Saha, A.; Lesins, G.; Duck, T. J.; Eloranta, E. W.; Nott, G. J.; Hoffman, A.; Karumudi, M. L.; Ritter, C.; Bourassa, A.; Abboud, I.; Carn, S. A.; Savastiouk, V.

    2012-02-01

    Aerosols from the Sarychev Peak volcano entered the Arctic region less than a week after the strongest SO2eruption on June 15 and 16, 2009 and had, by the first week in July, spread out over the entire Arctic region. These predominantly stratospheric aerosols were determined to be sub-micron in size and inferred to be composed of sulphates produced from the condensation of SO2gases emitted during the eruption. Average (500 nm) Sarychev-induced stratospheric optical depths (SOD) over the Polar Environmental Atmospheric Research Laboratory (PEARL) at Eureka (Nunavut, Canada) were found to be between 0.03 and 0.05 during the months of July and August, 2009. This estimate, derived from sunphotometry and integrated lidar backscatter profiles was consistent with averages derived from lidar estimates over Ny-Ålesund (Spitsbergen). The Sarychev SOD e-folding time at Eureka, deduced from lidar profiles, was found to be approximately 4 months relative to a regression start date of July 27. These profiles initially revealed the presence of multiple Sarychev plumes between the tropopause and about 17 km altitude. After about two months, the complex vertical plume structures had collapsed into fewer, more homogeneous plumes located near the tropopause. It was found that the noisy character of daytime backscatter returns induced an artifactual minimum in the temporal, pan-Arctic, CALIOP SOD response to Sarychev sulphates. A depolarization ratio discrimination criterion was used to separate the CALIOP stratospheric layer class into a low depolarization subclass which was more representative of Sarychev sulphates. Post-SAT (post Sarychev Arrival Time) retrievals of the fine mode effective radius (reff,f) and the logarithmic standard deviation for two Eureka sites and Thule (Greenland) were all close to 0.25 μm and 1.6 respectively. The stratospheric analogue to the columnar reff,f average was estimated to be reff,f(+) = 0.29 μm for Eureka data. Stratospheric, Raman lidar

  11. High Spectral Resolution Lidar and MPLNET Micro Pulse Lidar Aerosol Optical Property Retrieval Intercomparison During the 2012 7-SEAS Field Campaign at Singapore

    NASA Technical Reports Server (NTRS)

    Lolli, Simone; Welton, Ellsworth J.; Campbell, James R.; Eloranta, Edwin; Holben, Brent N.; Chew, Boon Ning; Salinas, Santo V.

    2014-01-01

    From August 2012 to February 2013 a High Resolution Spectral Lidar (HSRL; 532 nm) was deployed at that National University of Singapore near a NASA Micro Pulse Lidar NETwork (MPLNET; 527 nm) site. A primary objective of the MPLNET lidar project is the production and dissemination of reliable Level 1 measurements and Level 2 retrieval products. This paper characterizes and quantifies error in Level 2 aerosol optical property retrievals conducted through inversion techniques that derive backscattering and extinction coefficients from MPLNET elastic single-wavelength datasets. MPLNET Level 2 retrievals for aerosol optical depth and extinction/backscatter coefficient profiles are compared with corresponding HSRL datasets, for which the instrument collects direct measurements of each using a unique optical configuration that segregates aerosol and cloud backscattered signal from molecular signal. The intercomparison is performed, and error matrices reported, for lower (0-5km) and the upper (>5km) troposphere, respectively, to distinguish uncertainties observed within and above the MPLNET instrument optical overlap regime.

  12. Aerosol model development for environmental monitoring in the coastal atmosphere surface layer

    NASA Astrophysics Data System (ADS)

    Kaloshin, Gennady A.; Matvienko, Gennady G.

    2007-06-01

    Extinction of radiation in the marine boundary layer is dominated by scattering and absorption due to atmospheric aerosol. It is known, that the extinction of optical radiation visible and near IR spectra in the marine surface layer is determined mainly by scattering and absorption atmospheric aerosol. It influences on a dependence of spectral transmission and extinction both natural, and artificial light that is of interest for a wide range of problems, in particular for radiating problems at studying laws of climate formation, and for lines of the applications connected to the forecast of a signal power in coastal conditions at an estimation of EO systems characteristics. This is important to optical retrievals from satellite, remote sensing at environmental monitoring, backscatter of light to space (including climate forcing), cloud properties etc. In unpolluted regions the greatest effects on near shore scattering extinction will be a result of sea-salt from breaking waves and variations in relative humidity. The role of breaking waves appears to be modulated by wind, tide, swell, wave spectra and coastal conditions. These influences will be superimposed upon aerosol generated by open ocean sea-salt aerosol that varies with wind speed. The focus of our study is the extinction and optical effects due to aerosol in a specific coastal region. This involves linking coastal physical properties to oceanic and meteorological parameters in order to develop predictive algorithms that describe 3-D aerosol structure and variability. The aerosol microphysical model of the marine and coastal atmosphere surface layer is considered. The model distinctive feature is parameterization of amplitude and width of the modes as functions of fetch and wind speed. In the paper the dN/dr behavior depending at change meteorological parameters, heights above sea level, fetch, wind speed and RH is show. On the basis of the developed model with usage of Mie theory for spheres the

  13. Visibility related to backscatter at 1.54 micron

    NASA Technical Reports Server (NTRS)

    Barber, T. L.; Larson, D. R.

    1986-01-01

    The lidar process was shown to have the necessary potential to fulfill the need for a remote measurement of visibility. Visibility can be inferred from a lidar return optical extinction. The wavelength 1.54 micron was chosen, being near the visible wavelength region and having a high eye safety threshol, 200,000 times higher than 1.06 micron; 1.54 is the erbium laser wavelength. This research utilized 105 measured height profiles of natural droplet size distributions data, taken in clouds, fog, and haze. These profiles were examined to determine the completeness of the droplet counting data. It was found that the particle spectrometer data were incomplete in the very light ford and haze so this portion of the data was eliminated. Utilizing the Mie theory, these droplet size distribution profiles were converted to backscatter at 1.54 micron and extinction in the visible region, 0.55 micron. Using Koschmeider's relationship, the extinction profiles were converted to visibility. The visibility and backscatter profiles were compared to develop a relationship between visibility and backscatter at 1.54 micron.

  14. Aerosol remote sensing in polar regions

    SciTech Connect

    Tomasi, Claudio; Kokhanovsky, Alexander A.; Lupi, Angelo; Ritter, Christoph; Smirnov, Alexander; O'Neill, Norman T.; Stone, Robert S.; Holben, Brent N.; Nyeki, Stephan; Mazzola, Mauro; Lanconelli, Christian; Vitale, Vito; Stebel, Kerstin; Aaltonen, Veijo; de Leeuw, Gerrit; Rodriguez, Edith; Herber, Andreas B.; Radionov, Vladimir F.; Zielinski, Tymon; Petelski, Tomasz; Sakerin, Sergey M.; Kabanov, Dmitry M.; Xue, Yong; Mei, Linlu; Istomina, Larysa; Wagener, Richard; McArthur, Bruce; Sobolewski, Piotr S.; Kivi, Rigel; Courcoux, Yann; Larouche, Pierre; Broccardo, Stephen; Piketh, Stuart J.

    2015-01-01

    Multi-year sets of ground-based sun-photometer measurements conducted at 12 Arctic sites and 9 Antarctic sites were examined to determine daily mean values of aerosol optical thickness τ(λ) at visible and near-infrared wavelengths, from which best-fit values of Ångström's exponent α were calculated. Analysing these data, the monthly mean values of τ(0.50 μm) and α and the relative frequency histograms of the daily mean values of both parameters were determined for winter–spring and summer–autumn in the Arctic and for austral summer in Antarctica. The Arctic and Antarctic covariance plots of the seasonal median values of α versus τ(0.50 μm) showed: (i) a considerable increase in τ(0.50 μm) for the Arctic aerosol from summer to winter–spring, without marked changes in α; and (ii) a marked increase in τ(0.50 μm) passing from the Antarctic Plateau to coastal sites, whereas α decreased considerably due to the larger fraction of sea-salt aerosol. Good agreement was found when comparing ground-based sun-photometer measurements of τ(λ) and α at Arctic and Antarctic coastal sites with Microtops measurements conducted during numerous AERONET/MAN cruises from 2006 to 2013 in three Arctic Ocean sectors and in coastal and off-shore regions of the Southern Atlantic, Pacific, and Indian Oceans, and the Antarctic Peninsula. Lidar measurements were also examined to characterise vertical profiles of the aerosol backscattering coefficient measured throughout the year at Ny-Ålesund. Satellite-based MODIS, MISR, and AATSR retrievals of τ(λ) over large parts of the oceanic polar regions during spring and summer were in close agreement with ship-borne and coastal ground-based sun-photometer measurements. An overview of the chemical composition of mode particles is also presented, based on in-situ measurements at Arctic and Antarctic sites. Fourteen log-normal aerosol number size-distributions were defined to represent the average features of nuclei

  15. Aerosol remote sensing in polar regions

    DOE PAGES

    Tomasi, Claudio; Kokhanovsky, Alexander A.; Lupi, Angelo; Ritter, Christoph; Smirnov, Alexander; O'Neill, Norman T.; Stone, Robert S.; Holben, Brent N.; Nyeki, Stephan; Wehrli, Christoph; et al

    2015-01-01

    Multi-year sets of ground-based sun-photometer measurements conducted at 12 Arctic sites and 9 Antarctic sites were examined to determine daily mean values of aerosol optical thickness τ(λ) at visible and near-infrared wavelengths, from which best-fit values of Ångström's exponent α were calculated. Analysing these data, the monthly mean values of τ(0.50 μm) and α and the relative frequency histograms of the daily mean values of both parameters were determined for winter–spring and summer–autumn in the Arctic and for austral summer in Antarctica. The Arctic and Antarctic covariance plots of the seasonal median values of α versus τ(0.50 μm) showed: (i)more » a considerable increase in τ(0.50 μm) for the Arctic aerosol from summer to winter–spring, without marked changes in α; and (ii) a marked increase in τ(0.50 μm) passing from the Antarctic Plateau to coastal sites, whereas α decreased considerably due to the larger fraction of sea-salt aerosol. Good agreement was found when comparing ground-based sun-photometer measurements of τ(λ) and α at Arctic and Antarctic coastal sites with Microtops measurements conducted during numerous AERONET/MAN cruises from 2006 to 2013 in three Arctic Ocean sectors and in coastal and off-shore regions of the Southern Atlantic, Pacific, and Indian Oceans, and the Antarctic Peninsula. Lidar measurements were also examined to characterise vertical profiles of the aerosol backscattering coefficient measured throughout the year at Ny-Ålesund. Satellite-based MODIS, MISR, and AATSR retrievals of τ(λ) over large parts of the oceanic polar regions during spring and summer were in close agreement with ship-borne and coastal ground-based sun-photometer measurements. An overview of the chemical composition of mode particles is also presented, based on in-situ measurements at Arctic and Antarctic sites. Fourteen log-normal aerosol number size-distributions were defined to represent the average features of nuclei

  16. Aerosol Remote Sensing in Polar Regions

    NASA Technical Reports Server (NTRS)

    Tomasi, Claudio; Kokhanovsky, Alexander A.; Lupi, Angelo; Ritter, Christoph; Smirnov, Alexander; O'Neill, Norman T.; Stone, Robert S.; Holben, Brent N.; Nyeki, Stephan; Wehrli, Christoph

    2014-01-01

    Multi-year sets of ground-based sun-photometer measurements conducted at 12 Arctic sites and 9 Antarctic sites were examined to determine daily mean values of aerosol optical thickness tau(lambda) at visible and near-infrared wavelengths, from which best-fit values of Ångström's exponent alpha were calculated. Analyzing these data, the monthly mean values of tau(0.50 micrometers) and alpha and the relative frequency histograms of the daily mean values of both parameters were determined for winter-spring and summer-autumn in the Arctic and for austral summer in Antarctica. The Arctic and Antarctic covariance plots of the seasonal median values of alpha versus tau(0.50 micrometers) showed: (i) a considerable increase in tau(0.50 micrometers) for the Arctic aerosol from summer to winter-spring, without marked changes in alpha; and (ii) a marked increase in tau(0.50 micrometer) passing from the Antarctic Plateau to coastal sites, whereas alpha decreased considerably due to the larger fraction of sea-salt aerosol. Good agreement was found when comparing ground-based sun-photometer measurements of tau(lambda) and alpha at Arctic and Antarctic coastal sites with Microtops measurements conducted during numerous AERONET/MAN cruises from 2006 to 2013 in three Arctic Ocean sectors and in coastal and off-shore regions of the Southern Atlantic, Pacific, and Indian Oceans, and the Antarctic Peninsula. Lidar measurements were also examined to characterize vertical profiles of the aerosol backscattering coefficient measured throughout the year at Ny-Ålesund. Satellite-based MODIS, MISR, and AATSR retrievals of tau(lambda) over large parts of the oceanic polar regions during spring and summer were in close agreement with ship-borne and coastal ground-based sun-photometer measurements. An overview of the chemical composition of mode particles is also presented, based on in-situ measurements at Arctic and Antarctic sites. Fourteen log-normal aerosol number size-distributions were

  17. Some results of water vapor, ozone and aerosol balloon borne measurements during EASOE

    NASA Astrophysics Data System (ADS)

    Khattatov, V.; Yushkov, V.; Khaplanov, M.; Zaitzev, I.; Rosen, J.; Kjome, N.

    As part of the European Arctic Stratospheric Ozone Experiment (EASOE) in the northern winter of 1991/92, regular measurements of the vertical distribution of ozone and aerosols were carried out from two Russian polar stations, Heiss Island (81N, 58E) and Dikson Island (73N, 81E). In addition measurements of the vertical distribution of water vapor and aerosols were made from Esrange (68N, 21E), near Kiruna in Sweden. The instruments used were electrochemical ozone sondes (ECC-4A), a fluorescence hygrometer, and the University of Wyoming backscattersonde. Following the eruption of Mt.Pinatubo, in the Philippines, in June 1991, volcanic aerosol had reached Arctic latitudes at altitudes below 19 km by September. At all three sites it was observed on every flight. Polar stratospheric clouds were encountered above the volcanic aerosol on two flights from Esrange. There were no indications of dehydration in the Arctic stratosphere. On all flights the minimum mixing ratio of water vapor was observed 2 to 3 km above the tropopause. Total ozone was much lower than the climatological mean, over Dikson Island from the January 27, and over Heiss Island from mid-February, until the end of EASOE. Ozone profiles over these stations showed rapid increases in partial pressure immediately above the peak values of backscatter ratio when the volcanic aerosol was especially dense.

  18. Extinction-to-Backscatter Ratios of Saharan Dust Layers Derived from In-Situ Measurements and CALIPSO Overflights During NAMMA

    NASA Technical Reports Server (NTRS)

    Omar, Ali H.; Liu, Zhaoyan; Vaughan, Mark A.; Thornhill, Kenneth L., II; Kittaka, Chieko; Ismail, Syed; Chen, Gao; Powell, Kathleen A.; Winker, David M.; Trepte, Charles R.; Trepte, Charles R.; Winstead, Edward L.; Anderson, Bruce E.

    2010-01-01

    We determine the extinction-to-backscatter (Sa) ratios of dust using (1) airborne in-situ measurements of microphysical properties, (2) modeling studies, and (3) the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) observations recorded during the NASA African Monsoon Multidisciplinary Analyses (NAMMA) field experiment conducted from Sal, Cape Verde during Aug-Sept 2006. Using CALIPSO measurements of the attenuated backscatter of lofted Saharan dust layers, we apply the transmittance technique to estimate dust Sa ratios at 532 nm and a 2-color method to determine the corresponding 1064 nm Sa. This method yielded dust Sa ratios of 39.8 plus or minus 1.4 sr and 51.8 plus or minus 3.6 sr at 532 nm and 1064 nm, respectively. Secondly, Sa at both wavelengths is independently calculated using size distributions measured aboard the NASA DC-8 and estimates of Saharan dust complex refractive indices applied in a T-Matrix scheme. We found Sa ratios of 39.1 plus or minus 3.5 sr and 50.0 plus or minus 4 sr at 532 nm and 1064 nm, respectively, using the T-Matrix calculations applied to measured size spectra. Finally, in situ measurements of the total scattering (550 nm) and absorption coefficients (532 nm) are used to generate an extinction profile that is used to constrain the CALIPSO 532 nm extinction profile and thus generate a stratified 532 nm Sa. This method yielded an Sa ratio at 532 nm of 35.7 sr in the dust layer and 25 sr in the marine boundary layer consistent with a predominantly seasalt aerosol near the ocean surface. Combinatorial simulations using noisy size spectra and refractive indices were used to estimate the mean and uncertainty (one standard deviation) of these Sa ratios. These simulations produced a mean (plus or minus uncertainty) of 39.4 (plus or minus 5.9) sr and 56.5 (plus or minus 16.5) sr at 532 nm and 1064 nm, respectively, corresponding to percent uncertainties of 15% and 29%. These results will provide a measurements

  19. Aerosol in the Pacific troposphere

    NASA Technical Reports Server (NTRS)

    Clarke, Antony D.

    1989-01-01

    The use of near real-time optical techniques is emphasized for the measurement of mid-tropospheric aerosol over the Central Pacific. The primary focus is on measurement of the aerosol size distribution over the range of particle diameters from 0.15 to 5.0 microns that are essential for modeling CO2 backscatter values in support of the laser atmospheric wind sounder (LAWS) program. The measurement system employs a LAS-X (Laser Aerosol Spectrometer-PMS, Boulder, CO) with a custom 256 channel pulse height analyzer and software for detailed measurement and analysis of aerosol size distributions. A thermal preheater system (Thermo Optic Aerosol Descriminator (TOAD) conditions the aerosol in a manner that allows the discrimination of the size distribution of individual aerosol components such as sulfuric acid, sulfates and refractory species. This allows assessment of the relative contribution of each component to the BCO2 signal. This is necessary since the different components have different sources, exhibit independent variability and provide different BCO2 signals for a given mass and particle size. Field activities involve experiments designed to examine both temporal and spatial variability of these aerosol components from ground based and aircraft platforms.

  20. Airborne Sunphotometry of African Dust and Marine Boundary Layer Aerosols in PRIDE

    NASA Technical Reports Server (NTRS)

    Livingston, John M.; Redemann, Jens; Russell, Philip; Schmid, Beat; Reid, Jeff; Pilewskie, Peter; Hipskind, R. Stephen (Technical Monitor)

    2000-01-01

    The Puerto Rico Dust Experiment (PRIDE) was conducted during summer 2000 to study the radiative, microphysical and transport properties of Saharan dust in the Caribbean region. During PRIDE, NASA Ames Research Center's six-channel airborne autotracking sunphotometer (AATS-6) was operated aboard a Piper Navajo airplane based at Roosevelt Roads Naval Station on the northeast coast of Puerto Rico. AATS-6 measurements were taken during 21 science flights off the coast of Puerto Rico in the western Caribbean. Data were acquired within and above the Marine Boundary Layer (MBL) and the Saharan Aerosol Layer (SAL) up to 5.5 km altitude tinder a wide range of dust loadings. Aerosol optical depth (AOD) spectra and columnar water vapor (CWV) values have been calculated from the AATS-6 measurements by using sunphotometer calibration data obtained at Mauna Loa Observatory (3A kin ASL) before (May) and after (October) PRIDE. Mid-visible AOD values measured near the surface during PRIDE ranged from 0.07 on the cleanest day to 0.55 on the most turbid day. Values measured above the MBL were as high as 0.35; values above the SAL were as low as 0.01. The fraction of total column AOD due to Saharan dust cannot be determined precisely from AATS-6 AOD data alone due to the uncertainty in the extent of vertical mixing of the dust down through the MBL. However, analyses of ground-based and airborne in-situ aerosol sampling measurements and ground-based aerosol lidar backscatter data should yield accurate characterization of the vertical mixing that will enable calculation of the Saharan dust AOD component from the sunphotometer data. Examples will be presented showing measured AATS-6 AOD spectra, calculated aerosol extinction and water vapor density vertical profiles, and aerosol size distributions retrieved by inversion of the AOD spectra. Near sea-surface AOD spectra acquired by AATS-6 during horizontal flight legs at 30 m ASL are available for validation of AOD derived from coincident

  1. Study of aerosol microphysical properties profiles retrieved from ground-based remote sensing and aircraft in-situ measurements during a Saharan dust event

    NASA Astrophysics Data System (ADS)

    Granados-Muñoz, M. J.; Bravo-Aranda, J. A.; Baumgardner, D.; Guerrero-Rascado, J. L.; Pérez-Ramírez, D.; Navas-Guzmán, F.; Veselovskii, I.; Lyamani, H.; Valenzuela, A.; Olmo, F. J.; Titos, G.; Andrey, J.; Chaikovsky, A.; Dubovik, O.; Gil-Ojeda, M.; Alados-Arboledas, L.

    2015-09-01

    In this work we present an analysis of mineral dust optical and microphysical properties obtained from different retrieval techniques applied to active and passive remote sensing measurements, including a comparison with simultaneous in-situ aircraft measurements. Data were collected in a field campaign performed during a mineral dust outbreak a Granada, Spain, experimental site (37.16° N, 3.61° W, 680 m a.s.l.) on the 27 June 2011. Column-integrated properties are provided by sun- and star-photometry which allows a continuous evaluation of the mineral dust optical properties during both day and night-time. Both the Linear Estimation and AERONET (Aerosol Robotic Network) inversion algorithms are applied for the retrieval of the column-integrated microphysical particle properties. In addition, vertically-resolved microphysical properties are obtained from a multi-wavelength Raman lidar system included in EARLINET (European Aerosol Research Lidar Network), by using both LIRIC (Lidar Radiometer Inversion Code) algorithm during daytime and an algorithm applied to the Raman measurements based on the regularization technique during night-time. LIRIC retrievals reveal several dust layers between 3 and 5 km a.s.l. with volume concentrations of the coarse spheroid mode up to 60 μm3 cm-3. The combined use of the regularization and LIRIC methods reveals the night-to-day evolution of the vertical structure of the mineral dust microphysical properties and offers complementary information to that from column-integrated variables retrieved from passive remote sensing. Additionally, lidar depolarization profiles and LIRIC retrieved volume concentration are compared with aircraft in-situ measurements. This study presents for the first time a comparison of both volume concentration and dust particle polarization ratios measured with in-situ and remote sensing techniques. Results for the depolarization measurements in the dust layer indicate reasonable agreement within the

  2. Rayleigh-backscattering doppler broadening correction for differential absorption lidar

    NASA Astrophysics Data System (ADS)

    Fan, Lanlan; Zhang, Yinchao; Chen, Siying; Guo, Pan; Chen, He

    2015-11-01

    The spectral broadening by Rayleigh backscattering can cause large changes in water vapor echo signals, causing errors when the water vapor concentration is inversed by differential absorption lidar (DIAL). A correction algorithm is proposed to revise the errors due to the effect of laser spectral broadening. The relative errors of water vapor are calculated in cases of different aerosol distribution and temperature changes before and after correction. The results show that measurement errors due to the Doppler broadening are more than 5% before correction and a 2% measurement error after corrected for the case of a smooth, background aerosol distribution. However, due to the high aerosol gradients and strong temperature inversion, errors can be up to 40% and 10% with no corrections for this effect, respectively. The relative errors can reduce to less than 2% after correction. Hence, the correction algorithm for Rayleigh Doppler broadening can improve detection accuracy in H2O DIAL measurements especially when it is applied to high aerosol concentration or strong temperature inversion.

  3. Particle scattering, backscattering, and absorption coefficients: An in situ closure and sensitivity study

    NASA Astrophysics Data System (ADS)

    Wex, Heike; Neusüß, Christian; Wendisch, Manfred; Stratmann, Frank; Koziar, Christian; Keil, Andreas; Wiedensohler, Alfred; Ebert, Martin

    2002-11-01

    Comparisons between measured and calculated aerosol scattering, backscattering, and absorption coefficients were made based on in situ, ground-based measurements during the Melpitz INTensive (MINT) and Lindenberg Aerosol Characterization Experiment 1998 (LACE 98) field studies. Furthermore, airborne measurements made with the same type of instruments are reviewed and compared with the ground-based measurements. Agreement between measured and calculated values is on the order of ±20% for scattering and backscattering coefficients. A sensitivity analysis showed a large influence on the calculated particle scattering and backscattering coefficients resulting from sizing uncertainties in the measured number size distributions. Measured absorption coefficients were significantly smaller than the corresponding calculated values. The largest uncertainty for the calculated absorption coefficients resulted from the size-dependent fraction of elemental carbon (EC) of the aerosol. A correction for the measured fractions of EC could significantly improve the agreement between measured and calculated absorption coefficients. The overall uncertainty of the calculated values was investigated with a Monte Carlo method by simultaneously and randomly varying the input parameters of the calculations, where the variation of each parameter was bounded by its uncertainty. The measurements were mostly found to be within the range of uncertainties of the calculations, with uncertainties for the calculated scattering and backscattering coefficients of about ±20% and for the absorption coefficients of about ±30%. Thus, to increase the accuracy of calculated scattering, backscattering, and absorption coefficients, it is crucial to further reduce the error in particle number size distribution measurement techniques. In addition, further improvement of the techniques for measuring absorption coefficients and further investigation of the measurement of the fraction of EC of the aerosol is

  4. Stratospheric Aerosol Extinction Retrieval for SCIAMACHY Measurements in Limb Geometry

    NASA Astrophysics Data System (ADS)

    Dörner, S.; Pukite, J.; Penning de Vries, M.; Beirle, S.; Wagner, T.

    2015-12-01

    Techniques for retrieving height resolved information on stratospheric aerosol improved significantly in the past decade with the availability of satellites measurements in limb geometry. Instruments like OMPS, OSIRIS and SCIAMACHY provide height resolved radiance spectra with global coverage. Long term data sets of stratospheric aerosol extinction profiles are important for a detailed investigation of spatial and temporal variation and formation processes (e.g. after volcanic eruptions or in polar stratospheric clouds). Resulting data sets contain vital information for climate models (radiative effect) or chemistry models (reaction surface for heterogeneous chemistry). This study focuses on the SCIAMACHY instrument which measured scattered sunlight in the ultra violet, visible and near infra red spectral range between 2002 and 2012. SCIAMACHY's unique method of alternating measurements in limb and nadir geometry provides co-located profile and column information respectively that can be used to characterize plumes with small horizontal extents. The covered wavelength range potentially provides information on effective micro-physical properties of the aerosol particles. However, scattering on background aerosol constitutes only a small fraction of detected radiance and assumptions on particle characteristics (e.g., size distribution) have to be made which results in potential uncertainties especially for wavelengths below 700 nm and for measurements in backscatter geometry. Methods to reduce these uncertainties are investigated and applied to our newly developed retrieval algorithm. In addition, so called spatial straylight contamination of the measured signal was identified as a significant error source and an empirical correction scheme was developed. Comparisons with SAGE II measurement in occultation geometry and balloon borne measurements with an optical particle counter confirm the viability of our retrieval algorithm.

  5. Backscatter measurements for NIF ignition targets (invited)

    SciTech Connect

    Moody, J. D.; Datte, P.; Krauter, K.; Bond, E.; Michel, P. A.; Glenzer, S. H.; Divol, L.; Suter, L.; Meezan, N.; MacGowan, B. J.; Hibbard, R.; London, R.; Kilkenny, J.; Wallace, R.; Knittel, K.; Frieders, G.; Golick, B.; Ross, G.; Widmann, K.; Jackson, J.; and others

    2010-10-15

    Backscattered light via laser-plasma instabilities has been measured in early NIF hohlraum experiments on two beam quads using a suite of detectors. A full aperture backscatter system and near backscatter imager (NBI) instrument separately measure the stimulated Brillouin and stimulated Raman scattered light. Both instruments work in conjunction to determine the total backscattered power to an accuracy of {approx}15%. In order to achieve the power accuracy we have added time-resolution to the NBI for the first time. This capability provides a temporally resolved spatial image of the backscatter which can be viewed as a movie.

  6. Backscatter measurements for NIF ignition targets (invited).

    PubMed

    Moody, J D; Datte, P; Krauter, K; Bond, E; Michel, P A; Glenzer, S H; Divol, L; Niemann, C; Suter, L; Meezan, N; MacGowan, B J; Hibbard, R; London, R; Kilkenny, J; Wallace, R; Kline, J L; Knittel, K; Frieders, G; Golick, B; Ross, G; Widmann, K; Jackson, J; Vernon, S; Clancy, T

    2010-10-01

    Backscattered light via laser-plasma instabilities has been measured in early NIF hohlraum experiments on two beam quads using a suite of detectors. A full aperture backscatter system and near backscatter imager (NBI) instrument separately measure the stimulated Brillouin and stimulated Raman scattered light. Both instruments work in conjunction to determine the total backscattered power to an accuracy of ∼15%. In order to achieve the power accuracy we have added time-resolution to the NBI for the first time. This capability provides a temporally resolved spatial image of the backscatter which can be viewed as a movie.

  7. Atmospheric temperature profiling in the presence of clouds with a pure rotational Raman lidar by use of an interference-filter-based polychromator.

    PubMed

    Behrendt, A; Reichardt, J

    2000-03-20

    A lidar polychromator design for the measurement of atmospheric temperature profiles in the presence of clouds with the rotational Raman method is presented. The design utilizes multicavity interference filters mounted sequentially at small angles of incidence. Characteristics of this design are high signal efficiency and adjustable center wavelengths of the filters combined with a stable and relatively simple experimental setup. High suppression of the elastic backscatter signal in the rotational Raman detection channels allows temperature measurements independent of the presence of thin clouds or aerosol layers; no influence of particle scattering on the lidar temperature profile was observed in clouds with a backscatter ratio of at least 45. The minimum integration time needed for temperature profiling with a statistical temperature error of +/-1 K at, e.g., 20-km height and 960-m height resolution is 1.5 h.

  8. Metabolic Profiling as Well as Stable Isotope Assisted Metabolic and Proteomic Analysis of RAW 264.7 Macrophages Exposed to Ship Engine Aerosol Emissions: Different Effects of Heavy Fuel Oil and Refined Diesel Fuel.

    PubMed

    Sapcariu, Sean C; Kanashova, Tamara; Dilger, Marco; Diabaté, Silvia; Oeder, Sebastian; Passig, Johannes; Radischat, Christian; Buters, Jeroen; Sippula, Olli; Streibel, Thorsten; Paur, Hanns-Rudolf; Schlager, Christoph; Mülhopt, Sonja; Stengel, Benjamin; Rabe, Rom; Harndorf, Horst; Krebs, Tobias; Karg, Erwin; Gröger, Thomas; Weiss, Carsten; Dittmar, Gunnar; Hiller, Karsten; Zimmermann, Ralf

    2016-01-01

    Exposure to air pollution resulting from fossil fuel combustion has been linked to multiple short-term and long term health effects. In a previous study, exposure of lung epithelial cells to engine exhaust from heavy fuel oil (HFO) and diesel fuel (DF), two of the main fuels used in marine engines, led to an increased regulation of several pathways associated with adverse cellular effects, including pro-inflammatory pathways. In addition, DF exhaust exposure was shown to have a wider response on multiple cellular regulatory levels compared to HFO emissions, suggesting a potentially higher toxicity of DF emissions over HFO. In order to further understand these effects, as well as to validate these findings in another cell line, we investigated macrophages under the same conditions as a more inflammation-relevant model. An air-liquid interface aerosol exposure system was used to provide a more biologically relevant exposure system compared to submerged experiments, with cells exposed to either the complete aerosol (particle and gas phase), or the gas phase only (with particles filtered out). Data from cytotoxicity assays were integrated with metabolomics and proteomics analyses, including stable isotope-assisted metabolomics, in order to uncover pathways affected by combustion aerosol exposure in macrophages. Through this approach, we determined differing phenotypic effects associated with the different components of aerosol. The particle phase of diluted combustion aerosols was found to induce increased cell death in macrophages, while the gas phase was found more to affect the metabolic profile. In particular, a higher cytotoxicity of DF aerosol emission was observed in relation to the HFO aerosol. Furthermore, macrophage exposure to the gas phase of HFO leads to an induction of a pro-inflammatory metabolic and proteomic phenotype. These results validate the effects found in lung epithelial cells, confirming the role of inflammation and cellular stress in the

  9. Metabolic Profiling as Well as Stable Isotope Assisted Metabolic and Proteomic Analysis of RAW 264.7 Macrophages Exposed to Ship Engine Aerosol Emissions: Different Effects of Heavy Fuel Oil and Refined Diesel Fuel

    PubMed Central

    Sapcariu, Sean C.; Kanashova, Tamara; Dilger, Marco; Diabaté, Silvia; Oeder, Sebastian; Passig, Johannes; Radischat, Christian; Buters, Jeroen; Sippula, Olli; Streibel, Thorsten; Paur, Hanns-Rudolf; Schlager, Christoph; Mülhopt, Sonja; Stengel, Benjamin; Rabe, Rom; Harndorf, Horst; Krebs, Tobias; Karg, Erwin; Gröger, Thomas; Weiss, Carsten; Dittmar, Gunnar; Hiller, Karsten; Zimmermann, Ralf

    2016-01-01

    Exposure to air pollution resulting from fossil fuel combustion has been linked to multiple short-term and long term health effects. In a previous study, exposure of lung epithelial cells to engine exhaust from heavy fuel oil (HFO) and diesel fuel (DF), two of the main fuels used in marine engines, led to an increased regulation of several pathways associated with adverse cellular effects, including pro-inflammatory pathways. In addition, DF exhaust exposure was shown to have a wider response on multiple cellular regulatory levels compared to HFO emissions, suggesting a potentially higher toxicity of DF emissions over HFO. In order to further understand these effects, as well as to validate these findings in another cell line, we investigated macrophages under the same conditions as a more inflammation-relevant model. An air-liquid interface aerosol exposure system was used to provide a more biologically relevant exposure system compared to submerged experiments, with cells exposed to either the complete aerosol (particle and gas phase), or the gas phase only (with particles filtered out). Data from cytotoxicity assays were integrated with metabolomics and proteomics analyses, including stable isotope-assisted metabolomics, in order to uncover pathways affected by combustion aerosol exposure in macrophages. Through this approach, we determined differing phenotypic effects associated with the different components of aerosol. The particle phase of diluted combustion aerosols was found to induce increased cell death in macrophages, while the gas phase was found more to affect the metabolic profile. In particular, a higher cytotoxicity of DF aerosol emission was observed in relation to the HFO aerosol. Furthermore, macrophage exposure to the gas phase of HFO leads to an induction of a pro-inflammatory metabolic and proteomic phenotype. These results validate the effects found in lung epithelial cells, confirming the role of inflammation and cellular stress in the

  10. Metabolic Profiling as Well as Stable Isotope Assisted Metabolic and Proteomic Analysis of RAW 264.7 Macrophages Exposed to Ship Engine Aerosol Emissions: Different Effects of Heavy Fuel Oil and Refined Diesel Fuel.

    PubMed

    Sapcariu, Sean C; Kanashova, Tamara; Dilger, Marco; Diabaté, Silvia; Oeder, Sebastian; Passig, Johannes; Radischat, Christian; Buters, Jeroen; Sippula, Olli; Streibel, Thorsten; Paur, Hanns-Rudolf; Schlager, Christoph; Mülhopt, Sonja; Stengel, Benjamin; Rabe, Rom; Harndorf, Horst; Krebs, Tobias; Karg, Erwin; Gröger, Thomas; Weiss, Carsten; Dittmar, Gunnar; Hiller, Karsten; Zimmermann, Ralf

    2016-01-01

    Exposure to air pollution resulting from fossil fuel combustion has been linked to multiple short-term and long term health effects. In a previous study, exposure of lung epithelial cells to engine exhaust from heavy fuel oil (HFO) and diesel fuel (DF), two of the main fuels used in marine engines, led to an increased regulation of several pathways associated with adverse cellular effects, including pro-inflammatory pathways. In addition, DF exhaust exposure was shown to have a wider response on multiple cellular regulatory levels compared to HFO emissions, suggesting a potentially higher toxicity of DF emissions over HFO. In order to further understand these effects, as well as to validate these findings in another cell line, we investigated macrophages under the same conditions as a more inflammation-relevant model. An air-liquid interface aerosol exposure system was used to provide a more biologically relevant exposure system compared to submerged experiments, with cells exposed to either the complete aerosol (particle and gas phase), or the gas phase only (with particles filtered out). Data from cytotoxicity assays were integrated with metabolomics and proteomics analyses, including stable isotope-assisted metabolomics, in order to uncover pathways affected by combustion aerosol exposure in macrophages. Through this approach, we determined differing phenotypic effects associated with the different components of aerosol. The particle phase of diluted combustion aerosols was found to induce increased cell death in macrophages, while the gas phase was found more to affect the metabolic profile. In particular, a higher cytotoxicity of DF aerosol emission was observed in relation to the HFO aerosol. Furthermore, macrophage exposure to the gas phase of HFO leads to an induction of a pro-inflammatory metabolic and proteomic phenotype. These results validate the effects found in lung epithelial cells, confirming the role of inflammation and cellular stress in the

  11. Dust aerosol emission over the Sahara during summertime from Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) observations

    NASA Astrophysics Data System (ADS)

    Todd, Martin C.; Cavazos-Guerra, Carolina

    2016-03-01

    Dust aerosols are an important component of the climate system and a challenge to incorporate into weather and climate models. Information on the location and magnitude of dust emission remains a key information gap to inform model development. Inadequate surface observations ensure that satellite data remain the primary source of this information over extensive and remote desert regions. Here, we develop estimates of the relative magnitude of active dust emission over the Sahara desert based on data from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). Utilising the unique vertical profile of aerosol characteristics provided by CALIOP our algorithm identifies emission from aerosol extinction and lidar backscatter in the near surface layers. From the long-term CALIOP archive of day and night-time orbits over 2006-13 we construct coarse resolution maps of a new dust emission index (DEI) for the Sahara desert during the peak summer dust season (June to September). The spatial structure of DEI indicates highest emission over a broad zone focused on the border regions of Southern Algeria, Northern Mali and northwest Niger, displaced substantially (∼7°) to the east of the mean maximum in satellite-derived aerosol optical depth. In this region night-time emission exceeds that during the day. The DEI maps substantially corroborate recently derived dust source frequency count maps based on back-tracking plumes in high temporal resolution SEVIRI imagery. As such, a convergence of evidence from multiple satellite data sources using independent methods provides an increasingly robust picture of Saharan dust emission sources. Various caveats are considered. As such, quantitative estimates of dust emission may require a synergistic combined multi-sensor analysis.

  12. Backscatter absorption gas imaging system

    DOEpatents

    McRae, T.G. Jr.

    A video imaging system for detecting hazardous gas leaks. Visual displays of invisible gas clouds are produced by radiation augmentation of the field of view of an imaging device by radiation corresponding to an absorption line of the gas to be detected. The field of view of an imager is irradiated by a laser. The imager receives both backscattered laser light and background radiation. When a detectable gas is present, the backscattered laser light is highly attenuated, producing a region of contrast or shadow on the image. A flying spot imaging system is utilized to synchronously irradiate and scan the area to lower laser power requirements. The imager signal is processed to produce a video display.

  13. Backscatter absorption gas imaging system

    DOEpatents

    McRae, Jr., Thomas G.

    1985-01-01

    A video imaging system for detecting hazardous gas leaks. Visual displays of invisible gas clouds are produced by radiation augmentation of the field of view of an imaging device by radiation corresponding to an absorption line of the gas to be detected. The field of view of an imager is irradiated by a laser. The imager receives both backscattered laser light and background radiation. When a detectable gas is present, the backscattered laser light is highly attenuated, producing a region of contrast or shadow on the image. A flying spot imaging system is utilized to synchronously irradiate and scan the area to lower laser power requirements. The imager signal is processed to produce a video display.

  14. Electromagnetic backscattering by corner reflectors

    NASA Technical Reports Server (NTRS)

    Balanis, C. A.; Griesser, T.

    1986-01-01

    The Geometrical Theory of Diffraction (GTD), which supplements Geometric Optics (GO), and the Physical Theory of Diffraction (PTD), which supplements Physical Optics (PO), are used to predict the backscatter cross sections of dihedral corner reflectors which have right, obtuse, or acute included angles. These theories allow individual backscattering mechanisms of the dihedral corner reflectors to be identified and provide good agreement with experimental results in the azimuthal plane. The advantages and disadvantages of the geometrical and physical theories are discussed in terms of their accuracy, usefulness, and complexity. Numerous comparisons of analytical results with experimental data are presented. While physical optics alone is more accurate and more useful than geometrical optics alone, the combination of geometrical optics and geometrical diffraction seems to out perform physical optics and physical diffraction when compared with experimental data, especially for acute angle dihedral corner reflectors.

  15. Study of aerosol optical properties at Kunming in southwest China and long-range transport of biomass burning aerosols from North Burma

    NASA Astrophysics Data System (ADS)

    Zhu, J.; Xia, X.; Che, H.; Wang, J.; Zhang, J.; Duan, Y.

    2016-03-01

    Seasonal variation of aerosol optical properties and dominant aerosol types at Kunming (KM), an urban site in southwest China, is characterized. Substantial influences of the hygroscopic growth and long-range transport of biomass burning (BB) aerosols on aerosol optical properties at KM are revealed. These results are derived from a detailed analysis of (a) aerosol optical properties (e.g. aerosol optical depth (AOD), columnar water vapor (CWV), single scattering albedo (SSA) and size distribution) retrieved from sunphotometer measurements during March 2012-August 2013, (b) satellite AOD and active fire products, (c) the attenuated backscatter profiles from the space-born lidar, and (d) the back-trajectories. The mean AOD440nm and extinction Angstrom exponent (EAE440 - 870) at KM are 0.42 ± 0.32 and 1.25 ± 0.35, respectively. Seasonally, high AOD440nm (0.51 ± 0.34), low EAE440 - 870 (1.06 ± 0.34) and high CWV (4.25 ± 0.97 cm) during the wet season (May - October) contrast with their counterparts 0.17 ± 0.11, 1.40 ± 0.31 and 1.91 ± 0.37 cm during the major dry season (November-February) and 0.53 ± 0.29, 1.39 ± 0.19, and 2.66 ± 0.44 cm in the late dry season (March-April). These contrasts between wet and major dry season, together with the finding that the fine mode radius increases significantly with AOD during the wet season, suggest the importance of the aerosol hygroscopic growth in regulating the seasonal variation of aerosol properties. BB and Urban/Industrial (UI) aerosols are two major aerosol types. Back trajectory analysis shows that airflows on clean days during the major dry season are often from west of KM where the AOD is low. In contrast, air masses on polluted days are from west (in late dry season) and east (in wet season) of KM where the AOD is often large. BB air mass is found mostly originated from North Burma where BB aerosols are lifted upward to 5 km and then subsequently transported to southwest China via prevailing westerly winds.

  16. A Ground-Based 2-Micron DIAL System to Profile Tropospheric CO2 and Aerosol Distributions for Atmospheric Studies

    NASA Technical Reports Server (NTRS)

    Ismail, Syed; Koch, Grady; Abedin, Nurul; Refaat, Tamer; Rubio, Manuel; Davis, Kenneth; Miller, Charles; Singh, Upendra

    2006-01-01

    System will operate at a temperature insensitive CO2 line (2050.967 nm) with side-line tuning and off-set locking. Demonstrated an order of magnitude improvement in laser line locking needed for high precision measurements, side-line operation, and simultaneously double pulsing and line locking. Detector testing of phototransistor has demonstrated sensitivity to aerosol features over long distances in the atmosphere and resolve features approx. 100m. Optical systems that collect light onto small area detectors work well. Receiver optical designs are being optimized and data acquisition systems developed. CO2 line parameter characterization in progress In situ sensor calibration in progress for validation of DIAL CO2 system.

  17. New Lidar Capabilities in Space: An Overview of the Cloud-Aerosol Transport System (CATS)

    NASA Astrophysics Data System (ADS)

    McGill, M. J.; Yorks, J. E.; Hlavka, D. L.; Selmer, P. A.; Hart, W. D.; Palm, S. P.; Nowottnick, E. P.; Vaughan, M.; Rodier, S. D.; Colarco, P. R.; da Silva, A.; Buchard, V.

    2014-12-01

    The Cloud-Aerosol Transport System (CATS), built at NASA Goddard Space Flight Center as a payload for the International Space Station (ISS), is set to launch in the late 2014. CATS is an elastic backscatter lidar operating in one of three science modes with three wavelengths (1064, 532, 355 nm) and HSRL capability at 532 nm. Depolarization measurements will be made at the 532 and 1064 nm wavelengths. The CATS science modes are described in Figure 1. The ISS orbit is a 51 degree inclination orbit at an altitude of about 405 km. This orbit provides more comprehensive coverage of the tropics and mid-latitudes than sun-synchronous orbiting sensors, with nearly a three day repeat cycle. Thus, science applications of CATS include cloud and aerosol climate studies, air quality monitoring, and smoke/volcanic plume tracking. Current uncertainties in cloud and aerosol properties limit our ability to accurately model the Earth's climate system and predict climate change. These limitations are due primarily to difficulties in adequately measuring aerosols and clouds on a global scale. A primary science objectives of CATS is to provide global aerosol and cloud vertical profile data in near real time to for assimilation in aerosol transport models such as the NASA GEOS-5 model. Furthermore, the vertical profiles of cloud and aerosol properties provided by CATS will complement current and future passive satellite sensors. Another important science objective of CATS is to advance technology in support of future mission development. CATS will employ 355 nm and HSRL capabilities, as well as depolarization at multiple wavelengths. These expanded measurement capabilities will provide the science community with new and improved global data products that have yet to be retrieved from space-based lidar. In preparation for launch, simulations of the CATS lidar signal are produced using GEOS5 model data to develop and test future data products. An example of the simulated CATS attenuated

  18. Estimated desert-dust ice nuclei profiles from polarization lidar: methodology and case studies

    NASA Astrophysics Data System (ADS)

    Mamouri, R. E.; Ansmann, A.

    2015-03-01

    A lidar method is presented that permits the estimation of height profiles of ice nuclei concentrations (INC) in desert dust layers. The polarization lidar technique is applied to separate dust and non-dust backscatter and extinction coefficients. The desert dust extinction coefficients σd are then converted to aerosol particle number concentrations APC280 which consider particles with radius > 280 nm only. By using profiles of APC280 and ambient temperature T along the laser beam, the profile of INC can be estimated within a factor of 3 by means of APC-T-INC parameterizations from the literature. The observed close relationship between σd at 500 nm and APC280 is of key importance for a successful INC retrieval. We studied this link by means of AERONET (Aerosol Robotic Network) sun/sky photometer observations at Morocco, Cabo Verde, Barbados, and Cyprus during desert dust outbreaks. The new INC retrieval method is applied to lidar observations of dust layers with the spaceborne lidar CALIOP (Cloud Aerosol Lidar with Orthogonal Polarization) during two overpasses over the EARLINET (European Aerosol Research Lidar Network) lidar site of the Cyprus University of Technology (CUT), Limassol (34.7° N, 33° E), Cyprus. The good agreement between the CALIOP and CUT lidar retrievals of σd, APC280, and INC profiles corroborates the potential of CALIOP to provide 3-D global desert dust APC280 and INC data sets.

  19. Comparison of Aerosol Single Scattering Albedos Derived By Diverse Techniques in Two North Atlantic Experiments

    NASA Technical Reports Server (NTRS)

    Russell, P. B.; Redemann, J.; Schmid, B.; Bergstrom, R. W.; Livingston, J. M.; McIntosh, D. M.; Hartley, S.; Hobbs, P. V.; Quinn, P. K.; Carrico, C. M.; Hipskind, R. Stephen (Technical Monitor)

    2000-01-01

    Aerosol single scattering albedo w (the ratio of scattering to extinction) is important in determining aerosol climatic effects, in explaining relationships between calculated and measured radiative fluxes, and in retrieving aerosol optical depths from satellite radiances. Recently, two experiments in the North Atlantic region, TARFOX and ACE-2, determined aerosol w by a variety of techniques. The techniques included fitting of calculated to measured fluxes; retrievals of w from skylight radiances; best fits of complex refractive index to profiles of backscatter, extinction, and size distribution; and in situ measurements of scattering and absorption at the surface and aloft. Both TARFOX and ACE-2 found a fairly wide range of values for w at midvisible wavelengths, with 0.85 less than wmidvis less than 0.99 for the marine aerosol impacted by continental pollution. Frequency distributions of w could usually be approximated by lognormals in wmax-w, with some occurrence of bimodality, suggesting the influence of different aerosol sources or processing. In both TARFOX and ACE-2, closure tests between measured and calculated radiative fluxes yielded best-fit values of wmidvis of 0.90+/-0.04 for the polluted boundary layer. Although these results have the virtue of describing the column aerosol unperturbed by sampling, they are subject to questions about representativeness and possible artifacts (e.g., unknown gas absorption). The other techniques gave larger values for wmidvis for the polluted boundary layer, with a typical result of wmidvis = 0.95+/-0.04, Current uncertainties in vv are large in terms of climate effects. More tests are needed of the consistency among different methods and of humidification effects on w.

  20. MPL-Net Measurements of Aerosol and Cloud Vertical Distributions at Co-Located AERONET Sites

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth J.; Campbell, James R.; Berkoff, Timothy A.; Spinhirne, James D.; Tsay, Si-Chee; Holben, Brent; Starr, David OC. (Technical Monitor)

    2002-01-01

    In the early 1990s, the first small, eye-safe, and autonomous lidar system was developed, the Micropulse Lidar (MPL). The MPL acquires signal profiles of backscattered laser light from aerosols and clouds. The signals are analyzed to yield multiple layer heights, optical depths of each layer, average extinction-to-backscatter ratios for each layer, and profiles of extinction in each layer. In 2000, several MPL sites were organized into a coordinated network, called MPL-Net, by the Cloud and Aerosol Lidar Group at NASA Goddard Space Flight Center (GSFC) using funding provided by the NASA Earth Observing System. tn addition to the funding provided by NASA EOS, the NASA CERES Ground Validation Group supplied four MPL systems to the project, and the NASA TOMS group contributed their MPL for work at GSFC. The Atmospheric Radiation Measurement Program (ARM) also agreed to make their data available to the MPL-Net project for processing. In addition to the initial NASA and ARM operated sites, several other independent research groups have also expressed interest in joining the network using their own instruments. Finally, a limited amount of EOS funding was set aside to participate in various field experiments each year. The NASA Sensor Intercomparison and Merger for Biological and Interdisciplinary Oceanic Studies (SIMBIOS) project also provides funds to deploy their MPL during ocean research cruises. All together, the MPL-Net project has participated in four major field experiments since 2000. Most MPL-Net sites and field experiment locations are also co-located with sunphotometers in the NASA Aerosol Robotic Network. (AERONET). Therefore, at these locations data is collected on both aerosol and cloud vertical structure as well as column optical depth and sky radiance. Real-time data products are now available from most MPL-Net sites. Our real-time products are generated at times of AERONET aerosol optical depth (AOD) measurements. The AERONET AOD is used as input to our

  1. Temperature and humidity profiles in the atmosphere from spaceborne lasers: A feasibility study

    NASA Technical Reports Server (NTRS)

    Grassl, H.; Schluessel, P.

    1984-01-01

    Computer simulations of the differential absorption lidar technique in a space craft for the purpose of temperature and humidity profiling indicate: (1) Current technology applied to O2 and H2O lines in the .7 to .8 micrometers wavelength band gives sufficiently high signal-to-noise ratios (up to 50 for a single pulse pair) if backscattering by aerosol particles is high, i.e. profiling accurate to 2 K for temperature and 10% for humidity should be feasible within the turbid lower troposphere in 1 km layers and with an averaging over approximately 100 pulses. (2) The impact of short term fluctuations in aerosol particle concentration is too big for a one laser system. Only a two laser system firing at a time lag of about 1 millisecond can surmount these difficulties. (3) The finite width of the laser line and the quasi-random shift of this line introduce tolerable, partly systematic errors.

  2. Solution of multifrequency lidar inverse problem for a pre-set marine aerosol size-distribution formula

    SciTech Connect

    Piskozub, J.

    1994-12-31

    The multifrequency lidar inverse problem discussed consists of calculating the size distribution of sol particles from backscattered lidar data. Sea-water (marine) aerosol is particularly well suited for this kind of study as its scattering characteristics can be accurately represented by Mie theory as its particles are almost spherical and their complex index of refraction is well known. Here, a solution of the inverse problem concerning finding aerosol size distribution for a multifrequency lidar system working on a small number of wavelengths is proposed. The solution involves a best-fit method of finding parameters in a pre-set formula of particle size distribution. A comparison of results calculated with the algorithm from experimental lidar profiles with PMS data collected in Baltic Sea coastal zone is given.

  3. Observations of Smoke Aerosol from Biomass Burning in Mexico: Effect of Particle Aging on Radiative Forcing and Remote Sensing

    NASA Technical Reports Server (NTRS)

    Remer, Lorraine A.; Bruintjes, Roelof; Holben, Brent N.; Christopher, Sundar

    1999-01-01

    We take advantage of the May 1998 biomass burning event in Southern Mexico to test the global applicability of a smoke aerosol size model developed from data observed in South America. The Mexican event is an unique opportunity to observe well-aged, residual smoke. Observations of smoke aerosol size distribution made from vertical profiles of airborne in situ measurements show an inverse relationship between concentration and particle size that suggests the aging process continues more than a week after the smoke is separated from its fire sources. The ground-based radiometer retrievals show that the column-averaged, aged, Mexican smoke particles are larger (diameter = 0.28 - 0.33 micrometers) than the mean smoke particles in South America (diameter = 0.22 - 0.30 micrometers). However, the difference (delta - 0.06 micrometer) translates into differences in backscattering coefficient of only 4-7% and an increase of direct radiative forcing of only 10%.

  4. Multi-wavelength Airborne High Spectral Resolution Lidar Observations of Aerosol Above Clouds in California during DISCOVER-AQ

    NASA Astrophysics Data System (ADS)

    Hostetler, C. A.; Burton, S. P.; Ferrare, R. A.; Rogers, R. R.; Mueller, D.; Chemyakin, E.; Cook, A. L.; Harper, D. B.; Ziemba, L. D.; Beyersdorf, A. J.; Anderson, B. E.

    2013-12-01

    Accurately representing the vertical profile of aerosols is important for determining their radiative impact, which is still one of the biggest uncertainties in climate forcing. Aerosol radiative forcing can be either positive or negative depending on aerosol absorption properties and underlying albedo. Therefore, accurately characterizing the vertical distribution of aerosols, and specifically aerosols above clouds, is vital to understanding climate change. Unlike passive sensors, airborne lidar has the capability to make vertically resolved aerosol measurements of aerosols above and between clouds. Recently, NASA Langley Research Center has built and deployed the world's first airborne multi-wavelength High Spectral Resolution Lidar, HSRL-2. The HSRL-2 instrument employs the HSRL technique to measure extinction at both 355 nm and 532 nm and also measures aerosol depolarization and backscatter at 355 nm, 532 nm and 1064 nm. Additional HSRL-2 data products include aerosol type and range-resolved aerosol microphysical parameters (e.g., effective radius, number concentration, and single scattering albedo). HSRL-2 was deployed in the San Joaquin Valley, California, from January 16 to February 6, 2013, on the DISCOVER-AQ field campaign (Deriving Information on Surface Conditions from Column and Vertically Resolved Observations Relevant to Air Quality). On February 6, the observation region was mostly cloudy, and HSRL-2 saw two distinct aerosol layers above the clouds. One layer was aged boundary-layer pollution located just above cloud top at approximately 1.5 km above sea level. An aged smoke layer was also observed over land and over the ocean at altitudes 4-7 km ASL. In this study, we will show HSRL-2 products for these cases, and compare them with airborne in situ measurements of the 1.5-km layer from a coincident flight of the NASA P3B. We will also compare and contrast the HSRL-2 measurements of these two aerosol layers with each other and the clear-air boundary

  5. Radiative Effects of Aerosols

    NASA Technical Reports Server (NTRS)

    Valero, Francisco P. J.

    1996-01-01

    During the Atlantic Stratocumulus Transition Experiment (ASTEX) in June 1992, two descents in cloud-free regions allowed comparison of the change in aerosol optical depth as determined by an onboard total-direct-diffuse radiometer (TDDR) to the change calculated from measured size-resolved aerosol microphysics and chemistry. Both profiles included a pollution haze from Europe but the second also included the effect of a Saharan dust layer above the haze. The separate contributions of supermicrometer (coarse) and submicrometer (fine) aerosol were determined and thermal analysis of the pollution haze indicated that the fine aerosol was composed primarily of a sulfate/water mixture with a refractory soot-like core. The soot core increased the calculated extinction by about 10% in the most polluted drier layer relative to a pure sulfate aerosol but had significantly less effect at higher humidities. A 3 km descent through a boundary layer air mass dominated by pollutant aerosol with relative humidities (RH) 10-77% yielded a close agreement between the measured and calculated aerosol optical depths (550 nm) of 0.160 (+/- 0.07) and 0. 157 (+/- 0.034) respectively. During descent the aerosol mass scattering coefficient per unit sulfate mass varied from about 5 to 16 m(exp 2)/g and primarily dependent upon ambient RH. However, the total scattering coefficient per total fine mass was far less variable at about 4+/- 0.7 m(exp 2)/g. A subsequent descent through a Saharan dust layer located above the pollution aerosol layer revealed that both layers contributed similarly to aerosol optical depth. The scattering per unit mass of the coarse aged dust was estimated at 1.1 +/- 0.2 m(exp 2)/g. The large difference (50%) in measured and calculated optical depth for the dust layer exceeded measurements.

  6. Optical backscattering properties of the "clearest" natural waters

    NASA Astrophysics Data System (ADS)

    Twardowski, M. S.; Claustre, H.; Freeman, S. A.; Stramski, D.; Huot, Y.

    2007-11-01

    During the BIOSOPE field campaign October-December 2004, measurements of inherent optical properties from the surface to 500 m depth were made with a ship profiler at stations covering over 8000 km through the Southeast Pacific Ocean. Data from a ~3000 km section containing the very clearest waters in the central gyre are reported here. The total volume scattering function at 117°, βt(117°), was measured with a WET Labs ECO-BB3 sensor at 462, 532, and 650 nm with estimated uncertainties of 2×10-5, 5×10-6, and 2×10-6 m-1 sr-1, respectively. These values were approximately 6%, 3%, and 3% of the volume scattering by pure seawater at their respective wavelengths. From a methodological perspective, there were several results: - distributions were resolvable even though some of the values from the central gyre were an order of magnitude lower than the lowest previous measurements in the literature; - Direct in-situ measurements of instrument dark offsets were necessary to accurately resolve backscattering at these low levels; - accurate pure seawater backscattering values are critical in determining particulate backscattering coefficients in the open ocean (not only in these very clear waters); the pure water scattering values determined by Buiteveld et al. (1994) with a [1+0.3S/37] adjustment for salinity based on Morel (1974) appear to be the most accurate estimates, with aggregate accuracies as low as a few percent; and - closure was demonstrated with subsurface reflectance measurements reported by Morel et al. (2007) within instrument precisions, a useful factor in validating the backscattering measurements. This methodology enabled several observations with respect to the hydrography and the use of backscattering as a biogeochemical proxy: -The clearest waters sampled were found at depths between 300 and 350 m, from 23.5° S, 118° W to 26° S, 114° W, where total backscattering at 650 nm was not distinguishable from pure seawater; -Distributions of

  7. Optical backscattering properties of the "clearest" natural waters

    NASA Astrophysics Data System (ADS)

    Twardowski, M. S.; Claustre, H.; Freeman, S. A.; Stramski, D.; Huot, Y.

    2007-07-01

    During the BIOSOPE field campaign October-December 2004, measurements of inherent optical properties from the surface to 500 m depth were made with a ship profiler at stations covering over ~8000 km through the Southeast Pacific Ocean. Data from a ~3000 km section containing the very clearest waters in the central gyre are reported here. The total volume scattering function at 117°, βt(117°), was measured with a WET Labs ECO-BB3 sensor at 462, 532, and 650 nm with estimated uncertainties of 2×10-5, 5×10-6, and 2×10-6 m-1 sr-1, respectively. These values were approximately 6%, 3%, and 3% of the scattering by pure seawater at their respective wavelengths. From a methodological perspective, there were several results: - bbp distributions were resolvable even though some of the values from the central gyre were an order of magnitude lower than the lowest previous measurements in the literature; - Direct in-situ measurements of instrument dark offsets were necessary to accurately resolve backscattering at these low levels; - accurate pure seawater backscattering values are critical in determining particulate backscattering coefficients in the open ocean (not only in these very clear waters); the pure water scattering values determined by Buiteveld et al. (1994) with a [1 + 0.3S/37] adjustment for salinity based on Morel (1974) appear to be the most accurate estimates, with aggregate accuracies as low as a few percent; and - closure was demonstrated with subsurface reflectance measurements reported by Morel et al. (2007) within instrument precisions, a useful factor in validating the backscattering measurements. This methodology enabled several observations with respect to the hydrography and the use of backscattering as a biogeochemical proxy: - The clearest waters sampled were found at depths between 300 and 350 m, from 23.5° S, 118° W to 26° S, 114° W, where total backscattering at 650 nm was not distinguishable from pure seawater; - Distributions of

  8. Lidar Measurements of the Vertical Distribution of Aerosol Optical and Physical Properties over Central Asia

    DOE PAGES

    Chen, Boris B.; Sverdlik, Leonid G.; Imashev, Sanjar A.; Solomon, Paul A.; Lantz, Jeffrey; Schauer, James J.; Shafer, Martin M.; Artamonova, Maria S.; Carmichael, Gregory R.

    2013-01-01

    The vertical structure of aerosol optical and physical properties was measured by Lidar in Eastern Kyrgyzstan, Central Asia, from June 2008 to May 2009. Lidar measurements were supplemented with surface-based measurements of PM 2.5 and PM 10 mass and chemical composition in both size fractions. Dust transported into the region is common, being detected 33% of the time. The maximum frequency occurred in the spring of 2009. Dust transported to Central Asia comes from regional sources, for example, Taklimakan desert and Aral Sea basin, and from long-range transport, for example, deserts of Arabia, Northeast Africa, Iran, and Pakistan. Regionalmore » sources are characterized by pollution transport with maximum values of coarse particles within the planetary boundary layer, aerosol optical thickness, extinction coefficient, integral coefficient of aerosol backscatter, and minimum values of the Ångström exponent. Pollution associated with air masses transported over long distances has different characteristics during autumn, winter, and spring. During winter, dust emissions were low resulting in high values of the Ångström exponent (about 0.51) and the fine particle mass fraction (64%). Dust storms were more frequent during spring with an increase in coarse dust particles in comparison to winter. The aerosol vertical profiles can be used to lower uncertainty in estimating radiative forcing.« less

  9. Simulations of the observation of clouds and aerosols with the Experimental Lidar in Space Equipment system.

    PubMed

    Liu, Z; Voelger, P; Sugimoto, N

    2000-06-20

    We carried out a simulation study for the observation of clouds and aerosols with the Japanese Experimental Lidar in Space Equipment (ELISE), which is a two-wavelength backscatter lidar with three detection channels. The National Space Development Agency of Japan plans to launch the ELISE on the Mission Demonstrate Satellite 2 (MDS-2). In the simulations, the lidar return signals for the ELISE are calculated for an artificial, two-dimensional atmospheric model including different types of clouds and aerosols. The signal detection processes are simulated realistically by inclusion of various sources of noise. The lidar signals that are generated are then used as input for simulations of data analysis with inversion algorithms to investigate retrieval of the optical properties of clouds and aerosols. The results demonstrate that the ELISE can provide global data on the structures and optical properties of clouds and aerosols. We also conducted an analysis of the effects of cloud inhomogeneity on retrievals from averaged lidar profiles. We show that the effects are significant for space lidar observations of optically thick broken clouds.

  10. Project Overview: Cumulus Humilis Aerosol Processing Study (CHAPS): Proposed Summer 2007 ASP Field Campaign

    SciTech Connect

    Berkowitz, Carl M.; Berg, Larry K.; Ogren, J. A.; Hostetler, Chris A.; Ferrare, Richard

    2006-05-18

    This white paper presents the scientific motivation and preliminary logistical plans for a proposed ASP field campaign to be carried out in the summer of 2007. The primary objective of this campaign is to use the DOE Gulfstream-1 aircraft to make measurements characterizing the chemical, physical and optical properties of aerosols below, within and above large fields of fair weather cumulus and to use the NASA Langley Research Center’s High Spectral Resolution Lidar (HSRL) to make independent measurements of aerosol backscatter and extinction profiles in the vicinity of these fields. Separate from the science questions to be addressed by these observations will be information to add in the development of a parameterized cumulus scheme capable of including multiple cloud fields within a regional or global scale model. We will also be able to compare and contrast the cloud and aerosol properties within and outside the Oklahoma City plume to study aerosol processes within individual clouds. Preliminary discussions with the Cloud and Land Surface Interaction Campaign (CLASIC) science team have identified overlap between the science questions posed for the CLASIC Intensive Operation Period (IOP) and the proposed ASP campaign, suggesting collaboration would benefit both teams.

  11. Ice cloud backscatter study and comparison with CALIPSO and MODIS satellite data.

    PubMed

    Ding, Jiachen; Yang, Ping; Holz, Robert E; Platnick, Steven; Meyer, Kerry G; Vaughan, Mark A; Hu, Yongxiang; King, Michael D

    2016-01-11

    An invariant imbedding T-matrix (II-TM) method is used to calculate the single-scattering properties of 8-column aggregate ice crystals. The II-TM based backscatter values are compared with those calculated by the improved geometric-optics method (IGOM) to refine the backscattering properties of the ice cloud radiative model used in the MODIS Collection 6 cloud optical property product. The integrated attenuated backscatter-to-cloud optical depth (IAB-ICOD) relation is derived from simulations using a CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite) lidar simulator based on a Monte Carlo radiative transfer model. By comparing the simulation results and co-located CALIPSO and MODIS (Moderate Resolution Imaging Spectroradiometer) observations, the non-uniform zonal distribution of ice clouds over ocean is characterized in terms of a mixture of smooth and rough ice particles. The percentage of the smooth particles is approximately 6% and 9% for tropical and midlatitude ice clouds, respectively.

  12. Development of a global backscatter model for NASA's laser atmospheric wind sounder

    NASA Technical Reports Server (NTRS)

    Bowdle, David; Collins, Laurie; Mach, Douglas; Mcnider, Richard; Song, Aaron

    1992-01-01

    During the Contract Period April 1, 1989, to September 30, 1992, the Earth Systems Science Laboratory (ESSL) in the Research Institute at the University of Alabama in Huntsville (UAH) conducted a program of basic research on atmospheric backscatter characteristics, leading to the development of a global backscatter model. The ESSL research effort was carried out in conjunction with the Earth System Observing Branch (ES43) at the National Aeronautics and Space Administration (NASA) Marshall Space Flight Center, as part of NASA Contract NAS8-37585 under the Atmospheric Dynamics Program at NASA Headquarters. This research provided important inputs to NASA's GLObal Backscatter Experiment (GLOBE) program, especially in the understanding of global aerosol life cycles, and to NASA's Doppler Lidar research program, especially the development program for their prospective space-based Laser Atmospheric Wind Sounder (LAWS).

  13. Aerosol Optical Thickness comparisons between NASA LaRC Airborne HSRL and AERONET during the DISCOVER-AQ field campaigns

    NASA Astrophysics Data System (ADS)

    Scarino, A. J.; Ferrare, R. A.; Burton, S. P.; Hostetler, C. A.; Hair, J. W.; Rogers, R. R.; Berkoff, T.; Cook, A. L.; Harper, D. B.; Hoff, R. M.; Holben, B. N.; Schafer, J.; McGill, M. J.; Yorks, J. E.; Lantz, K. O.; Michalsky, J. J.; Hodges, G.

    2013-12-01

    The first- and second-generation NASA airborne High Spectral Resolution Lidars (HSRL-1 and HSRL-2) have been deployed on board the NASA Langley Research Center King Air aircraft during the Deriving Information on Surface Conditions from Column and VERtically Resolved Observations Relevant to Air Quality (DISCOVER-AQ) field campaigns. These included deployments during July 2011 over Washington, D.C. and Baltimore, MD and during January and February 2013 over the San Joaquin Valley (SJV) of California and also a scheduled deployment during September 2013 over Houston, TX. Measurements of aerosol extinction, backscatter, and depolarization are available from both HSRL-1 and HSRL-2 in coordination with other participating research aircraft and ground sites. These measurements constitute a diverse data set for use in characterizing the spatial and temporal distribution of aerosols, aerosol optical thickness (AOT), as well as the Mixing Layer Height (MLH). HSRL AOT is compared to AOT measured by the Distributed Regional Aerosol Gridded Observation Networks (DRAGON) and long-term AERONET sites. For the 2011 campaign, comparisons of AOT at 532nm between HSRL-1 and AERONET showed excellent agreement (r = 0.98, slope = 1.01, intercept = 0.037) when the King Air flights were within 2.5 km of the ground site and 10 min from the retrieval time. The comparison results are similar for the 2013 DISCOVER-AQ campaign in the SJV. Additional ground-based (MPL) and airborne (CPL) lidar data were used to help screen for clouds in the AERONET observations during the SJV portion. AOT values from a Multi-Filter Rotating Shadowband Radiometer (MFRSR) located at the Porterville, CA site during the SJV campaign are also compared to HSRL-2 AOT. Lastly, using the MLH retrieved from HSRL aerosol backscatter profiles, we describe the distribution of AOT relative to the MLH.

  14. Future Mission Concept for 3-D Aerosol Monitoring From Space Based on Fusion of Remote Sensing Approaches

    NASA Astrophysics Data System (ADS)

    Diner, D. J.; Kahn, R. A.; Hostetler, C. A.; Ferrare, R. A.; Hair, J. W.; Cairns, B.; Torres, O.

    2006-05-01

    Fine airborne particles are implicated in adverse impacts on human health. In situ measurements are a critical component of any air quality monitoring system; however, they cover a small fraction of the globe and do not measure aerosols transported aloft or over water. Satellites provide a substantial complementary role, and great strides in aerosol characterization over land from spaceborne platforms are currently taking place. In the passive realm, multiangle sensors such as MISR have unique strengths in determining particle optical depths over land, constraining column-average particle size, shape, and single-scattering albedo, and providing stereoscopic layer-top heights for aerosol plumes and spatially heterogeneous layers. Multispectral information at ultraviolet (UV) wavelengths (e.g., from TOMS and OMI) and in the shortwave infrared (SWIR) (e.g., from MODIS), as well as polarimetry (e.g., from POLDER and in the future, APS) have complementary strengths for measuring aerosol microphysical properties. Active lidars bring added sensitivity to particle vertical distribution. Fusion of such capabilities, particularly at km-scale resolutions required for aerosol monitoring in urban settings, would further improve our ability to identify and track aerosol air mass types on regional and larger scales, giving added value and context to more detailed particle microphysical and chemical properties that can be measured in situ. In 2005 we submitted a mission concept called the Aerosol Global Interactions Satellite (AEGIS), consisting of a notional multiangle spectropolarimetric imager (MSPI) and high spectral resolution lidar (HSRL), to the National Academy of Sciences Decadal Survey. The MSPI instrument is an advanced version of MISR, improving upon current capabilities by adding near-UV, SWIR, and high-accuracy polarimetric imaging channels, and by widening the sensor swath. HSRL measurements are designed to provide vertical profiles of aerosol backscatter and

  15. Vertical Profiles of Light Scattering, Light Absorption, and Single Scattering Albedo during the Dry, Biomass Burning Season in Southern Africa and Comparisons of In Situ and Remote Sensing Measurements of Aerosol Optical Depths

    NASA Technical Reports Server (NTRS)

    Magi, Brian I.; Hobbs, Peter V.; Schmid, Beat; Redermann, Jens

    2003-01-01

    Airborne in situ measurements of vertical profiles of aerosol light scattering, light absorption, and single scattering albedo (omega (sub 0)) are presented for a number of locations in southern Africa during the dry, biomass burning season. Features of the profiles include haze layers, clean air slots, and marked decreases in light scattering in passing from the boundary layer into the free troposphere. Frequency distributions of omega (sub 0) reflect the strong influence of smoke from biomass burning. For example, during a period when heavy smoke was advected into the region from the north, the mean value of omega (sub 0) in the boundary layer was 0.81 +/- 0.02 compared to 0.89 +/- 0.03 prior to this intrusion. Comparisons of layer aerosol optical depths derived from the in situ measurements with those measured by a Sun photometer aboard the aircraft show excellent agreement.

  16. Raman-lidar technique for tropospheric and stratospheric sensing of aerosol optical and microphysical properties

    SciTech Connect

    Wandinger, U.

    1995-01-01

    Tropospheric and stratospheric aerosols and clouds are known to influence the earth`s radiation budget as well as chemical processes of the atmosphere. Thus, remote sensing of optical and microphysical properties of atmospheric particles has important applications in weather and climate research, pollution monitoring, and atmospheric chemistry. During the last few years Raman lidars have become very important tools in this field of research. The development of powerful light sources such as Nd:YAG and excimer lasers, of interference filters with narrow bandwidth and high transmission, and of low-noise photomultiplier tubes and counting systems has improved the Raman-lidar technique during the past decade significantly. The technique is based on the detection of two signals resulting from elastic backscattering by air molecules and particles and inelastic (Raman) backscattering by a gas of known number density, i.e., nitrogen or oxygen. The technique has been successfully applied to cirrus-cloud studies. In this presentation, the capability of the Raman-lidar technique for tropospheric and stratospheric profiling of aerosol and cloud properties will be discussed on the basis of measurement examples.

  17. On Backscatter in Ocean Dynamics

    NASA Astrophysics Data System (ADS)

    Nadiga, Balasubramanya

    2010-05-01

    Downgradient mixing of potential-voriticity and its variants are commonly employed to model the effects of unresolved geostrophic turbulence on resolved scales. This is motivated by the (inviscid and unforced) particle-wise conservation of potential-vorticity and the mean forward or down-scale cascade of potential enstrophy in geostrophic turubulence. By examining the statistical distribution of the transfer of potential enstrophy from mean or filtered motions to eddy or sub-filter motions, we find that the mean forward cascade results from the forward-scatter being only slightly greater than the backscatter. Downgradient mixing ideas, do not recognize such equitable mean-eddy or large scale-small scale interactions and consequently model only the mean effect of forward cascade. Consequently, we consider two alternate approaches to modeling backscatter---one based on the Large Eddy Simulation approach and the other based on regularization approach. We demonstrate the equivalence of the two approaches in a certain limit and present results that use the new parameterizations.

  18. Comparison of the aerosol optical properties and size distribution retrieved by sun photometer with in situ measurements at midlatitude

    NASA Astrophysics Data System (ADS)

    Chauvigné, Aurélien; Sellegri, Karine; Hervo, Maxime; Montoux, Nadège; Freville, Patrick; Goloub, Philippe

    2016-09-01

    Aerosols influence the Earth radiative budget through scattering and absorption of solar radiation. Several methods are used to investigate aerosol properties and thus quantify their direct and indirect impacts on climate. At the Puy de Dôme station, continuous high-altitude near-surface in situ measurements and low-altitude ground-based remote sensing atmospheric column measurements give the opportunity to compare the aerosol extinction measured with both methods over a 1-year period. To our knowledge, it is the first time that such a comparison is realised with continuous measurements of a high-altitude site during a long-term period. This comparison addresses to which extent near-surface in situ measurements are representative of the whole atmospheric column, the aerosol mixing layer (ML) or the free troposphere (FT). In particular, the impact of multi-aerosol layers events detected using lidar backscatter profiles is analysed. A good correlation between in situ aerosol extinction coefficient and aerosol optical depth (AOD) measured by the Aerosol Robotic Network (AERONET) sun photometer is observed with a correlation coefficient around 0.80, indicating that the in situ measurements station is representative of the overall atmospheric column. After filtering for multilayer cases and correcting for each layer optical contribution (ML and FT), the atmospheric structure seems to be the main factor influencing the comparison between the two measurement techniques. When the site lies in the ML, the in situ extinction represents 45 % of the sun photometer ML extinction while when the site lies within the FT, the in situ extinction is more than 2 times higher than the FT sun photometer extinction. Moreover, the assumption of a decreasing linear vertical aerosol profile in the whole atmosphere has been tested, significantly improving the instrumental agreement. Remote sensing retrievals of the aerosol particle size distributions (PSDs) from the sun photometer

  19. A self-directing elastic backscatter lidar system for debris cloud tracking and characterization

    SciTech Connect

    Clark, D.A.; Dighe, K.A.; Tunnell, T.W.

    1996-06-01

    An elastic backscatter lidar that utilizes the lidar signal itself to direct the system towards fast moving isolated aerosol clouds has been developed. However, detecting and tracking invisible transient effluents from unknown locations, though conceptually straightforward, has still remained experimentally challenging. Accurate cloud volume, cloud density distribution, and track information have been obtained on small, fast moving, subvisible debris clouds resulting from above ground tests in which conventional explosives were detonated.

  20. Inter-comparison of MAX-DOAS Retrieved Vertical Profiles of Aerosol Extinction, SO2 and NO2 in the Alberta Oil Sands with LIDAR Data and GEM-MACH Air Quality Model.

    NASA Astrophysics Data System (ADS)

    Davis, Zoe; Friess, Udo; Strawbridge, Kevin; Whiteway, James; Aggarwal, Monika; Makar, Paul; Li, Shao-Meng; O'Brien, Jason; Baray, Sabour; Schnitzler, Elijah; Olfert, Jason S.; Osthoff, Hans D.; Lobo, Akshay; McLaren, Robert

    2016-04-01

    Understanding industrial emissions of trace gas pollutants in the Alberta oil sands is essential to maintaining air quality standards and informing public policy. Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) measurements of trace gases can improve knowledge of pollutant levels, vertical distribution and chemical transformation. During an intensive air measurement campaign to study emissions, transport, transformation and deposition of oil sands air pollutants from August to September of 2013, a MAX-DOAS instrument was deployed at a site north of Fort McMurray, Alberta to determine the vertical profiles of aerosol extinction, NO2 and SO2 through retrieval from the MAX-DOAS spectral measurements using an optimal estimation method. The large complement of data collected from multiple instruments deployed during this field campaign provides a unique opportunity to validate and characterize the performance of the MAX-DOAS vertical profile retrievals. Aerosol extinction profiles determined from two Light Detection and Ranging (LIDAR) instruments, one collocated and the other on a Twin Otter aircraft that flew over the site during the study, will be compared to the MAX-DOAS aerosol extinction profile retrievals. Vertical profiles of NO2 and SO2 retrieved from the MAX-DOAS measurements will be further compared with the composite vertical profiles measured from the flights of a second aircraft, the NRC-Convair 580, over the field site during the same measurement period. Finally, the MAX-DOAS retrieved tropospheric vertical column densities (VCDs) of SO2 and NO2 will be compared to the predicted VCDs from Environment and Climate Change Canada's Global Environmental Multi-scale - Modelling Air quality and Chemistry (GEM-MACH) air quality model over the grid cell containing the field site. Emission estimates of SO2 from the major oil mining facility Syncrude Mildred Lake using the MAX-DOAS VCD results, validated through the detailed characterization above

  1. Cloud-Aerosol Interactions: Retrieving Aerosol Ångström Exponents from Calipso Measurements of Opaque Water Clouds

    NASA Astrophysics Data System (ADS)

    Vaughan, Mark; Liu, Zhaoyan; Hu, Yong-Xiang; Powell, Kathleen; Omar, Ali; Rodier, Sharon; Hunt, William; Kar, Jayanta; Tackett, Jason; Getzewich, Brian; Lee, Kam-Pui

    2016-06-01

    Backscatter and extinction from water clouds are well-understood, both theoretically and experimentally, and thus changes to the expected measurement of layer-integrated attenuated backscatter can be used to infer the optical properties of overlying layers. In this paper we offer a first look at a new retrieval technique that uses CALIPSO measurements of opaque water clouds to derive optical depths and Ångström exponents for overlying aerosol layers.

  2. Combining Passive Polarimetric and Lidar Observations from TCAP to Vertically Partition a Multi-Modal Aerosol Model

    NASA Astrophysics Data System (ADS)

    Cairns, B.; Ottaviani, M.; Knobelspiesse, K. D.; Chowdhary, J.; Hostetler, C. A.; Ferrare, R. A.; Hair, J. W.; Cook, A. L.; Harper, D. B.; Mack, T. L.; Hare, R. J.; Cleckner, C. S.; Rogers, R.; Mueller, D.; Burton, S. P.; Obland, M. D.; Scarino, A. J.; Redemann, J.; Schmid, B.; Fast, J. D.; Berg, L. K.

    2012-12-01

    The first airborne deployment associated with the Two-Column Aerosol Project (TCAP) field campaign was carried out on Cape Cod, Massachusetts during July 2012 using the DOE Gulfstream 1 (G-1) and the NASA Langley B200. The first column located on Cape Cod has the surface based ARM Mobile Facility, which measures aerosol properties, radiation, and cloud characteristics, as its anchor point. The second column, 200 km to the East, was chosen to facilitate characterization of the large gradient of AOD near the coast of New England. The G-1 was equipped with a suite of in situ instrumentation to measure the size, composition and optics of aerosols, together with spectral Aerosol Optical Depth (AOD) above the aircraft using the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research. The G1 generally flew at low altitude except when profiling the two columns. The B200, flew at ~ 9 km, above the G1, and operated the world's first airborne three backscatter (355, 532 and 1064 nm) and two extinction (355 and 532 nm) channel high-spectral-resolution lidar, HSRL-2 and the Research Scanning Polarimeter (RSP), which provides multi-angle multi-spectral observations of the intensity and polarization over a spectral range from 410 to 2260 nm. The TCAP measurements are ideal for remote sensing of aerosols since a dark ocean allows the full power of the passive intensity and polarization observations to be explored. RSP observations over the ocean have previously been used to retrieve the AOD, particle size and complex refractive index of aerosols, but it was noted that the vertical distribution of the aerosols could affect the accuracy of the retrieval. In this paper we combine HSRL-2 and RSP data to retrieve and partition a multi-modal aerosol model through the column. The lidar intensive variables (ratios of the lidar observations) that do not depend on aerosol load are used to constrain the microphysics of the aerosol modes. Where the classification technique presented

  3. Organic aerosols

    SciTech Connect

    Penner, J.E.

    1994-01-01

    Organic aerosols scatter solar radiation. They may also either enhance or decrease concentrations of cloud condensation nuclei. This paper summarizes observed concentrations of aerosols in remote continental and marine locations and provides estimates for the sources of organic aerosol matter. The anthropogenic sources of organic aerosols may be as large as the anthropogenic sources of sulfate aerosols, implying a similar magnitude of direct forcing of climate. The source estimates are highly uncertain and subject to revision in the future. A slow secondary source of organic aerosols of unknown origin may contribute to the observed oceanic concentrations. The role of organic aerosols acting as cloud condensation nuclei (CCN) is described and it is concluded that they may either enhance or decrease the ability of anthropogenic sulfate aerosols to act as CCN.

  4. Beta Backscatter Measures the Hardness of Rubber

    NASA Technical Reports Server (NTRS)

    Morrissey, E. T.; Roje, F. N.

    1986-01-01

    Nondestructive testing method determines hardness, on Shore scale, of room-temperature-vulcanizing silicone rubber. Measures backscattered beta particles; backscattered radiation count directly proportional to Shore hardness. Test set calibrated with specimen, Shore hardness known from mechanical durometer test. Specimen of unknown hardness tested, and radiation count recorded. Count compared with known sample to find Shore hardness of unknown.

  5. Estimation of volcanic ash emission profiles using ceilometer measurements and transport models

    NASA Astrophysics Data System (ADS)

    Chan, Ka Lok; Geiß, Alexander; Gasteiger, Josef; Wagner, Frank; Wiegner, Matthias

    2016-04-01

    In recent years, the number of active remote sensing systems grows rapidly, since several national weather services initiated ceilometer networks. These networks are excellent tools to monitor the dispersion of volcanic ash clouds and to validate chemical transport models. Moreover, it is expected that the can be used to refine model calculations to better predict situations that might be dangerous for aviation. As a ceilometer can be considered as a simple single-wavelength backscatter lidar, quantitative aerosol profile information, i.e., the aerosol backscatter coefficient (βp) profile, can be derived provided that the ceilometer is calibrated. Volcanic ash concentration profile can then be estimated by using prior optical properties of volcanic ash. These profiles are then used for the inverse calculation of the emission profile of the volcanic eruption, thus, improving one of the most critical parameters of the numerical simulation. In this study, the Lagrangian particle dispersion model FLEXPART (FLEXible PARTicle dispersion model) is used to simulate the dispersion of volcanic ash. We simulate the distribution of ash for a given time/height grid, in order to compute the sensitivity functions for each measurements. As an example we use ceilometer measurements of the German weather service to reconstruct the temporal and spatial emission profile of Eyjafjallajökull eruption in April 2010. We have also examined the sensitivity of the retrieved emission profiles to different measurement parameters, e.g., geolocation of the measurement sites, total number of measurement sites, temporal and vertical resolution of the measurements, etc. The first results show that ceilometer measurements in principle are feasible for the inversion of volcanic ash emission profiles.

  6. Cloud-Driven Changes in Aerosol Optical Properties - Final Technical Report

    SciTech Connect

    Ogren, John A.; Sheridan, Patrick S.; Andrews, Elisabeth

    2007-09-30

    The optical properties of aerosol particles are the controlling factors in determining direct aerosol radiative forcing. These optical properties depend on the chemical composition and size distribution of the aerosol particles, which can change due to various processes during the particles’ lifetime in the atmosphere. Over the course of this project we have studied how cloud processing of atmospheric aerosol changes the aerosol optical properties. A counterflow virtual impactor was used to separate cloud drops from interstitial aerosol and parallel aerosol systems were used to measure the optical properties of the interstitial and cloud-scavenged aerosol. Specifically, aerosol light scattering, back-scattering and absorption were measured and used to derive radiatively significant parameters such as aerosol single scattering albedo and backscatter fraction for cloud-scavenged and interstitial aerosol. This data allows us to demonstrate that the radiative properties of cloud-processed aerosol can be quite different than pre-cloud aerosol. These differences can be used to improve the parameterization of aerosol forcing in climate models.

  7. Cloud Scavenging Effects on Aerosol Radiative and Cloud-nucleating Properties - Final Technical Report

    SciTech Connect

    Ogren, John A.; Sheridan, Patrick S.; Andrews, Elisabeth

    2009-03-05

    The optical properties of aerosol particles are the controlling factors in determining direct aerosol radiative forcing. These optical properties depend on the chemical composition and size distribution of the aerosol particles, which can change due to various processes during the particles’ lifetime in the atmosphere. Over the course of this project we have studied how cloud processing of atmospheric aerosol changes the aerosol optical properties. A counterflow virtual impactor was used to separate cloud drops from interstitial aerosol and parallel aerosol systems were used to measure the optical properties of the interstitial and cloud-scavenged aerosol. Specifically, aerosol light scattering, back-scattering and absorption were measured and used to derive radiatively significant parameters such as aerosol single scattering albedo and backscatter fraction for cloud-scavenged and interstitial aerosol. This data allows us to demonstrate that the radiative properties of cloud-processed aerosol can be quite different than pre-cloud aerosol. These differences can be used to improve the parameterization of aerosol forcing in climate models.

  8. CALIPSO Observations of Volcanic Aerosol in the Stratosphere

    NASA Technical Reports Server (NTRS)

    Thomason, Larry W.; Pitts, Michael C.

    2008-01-01

    In the stratosphere, the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) has observed the presence of aerosol plumes associated with the eruptions several volcanoes including Montserrat (May 2006), Chaiten (May 2008), and Kasatochi (August 2008). While the dense ash plumes from these eruptions dissipate relatively quickly, CALIPSO continued to detect an enhanced aerosol layer from the Montserrat eruption from the initial observations in June 2006 well into 2008. Solar occultation missions were uniquely capable of monitoring stratospheric aerosol. However, since the end of long-lived instruments like the Stratospheric Aerosol and Gas Experiment (SAGE II), there has been no clear space-based successor instrument. A number of active instruments, some employing new techniques, are being evaluated as candidate sources of stratospheric aerosol data. Herein, we examine suitability of the CALIPSO 532-nm aerosol backscatter coefficient measurements.

  9. Lidar backscatter signal recovery from phototransistor systematic effect by deconvolution.

    PubMed

    Refaat, Tamer F; Ismail, Syed; Abedin, M Nurul; Spuler, Scott M; Mayor, Shane D; Singh, Upendra N

    2008-10-10

    Backscatter lidar detection systems have been designed and integrated at NASA Langley Research Center using IR heterojunction phototransistors. The design focused on maximizing the system signal-to-noise ratio rather than noise minimization. The detection systems have been validated using the Raman-shifted eye-safe aerosol lidar (REAL) at the National Center for Atmospheric Research. Incorporating such devices introduces some systematic effects in the form of blurring to the backscattered signals. Characterization of the detection system transfer function aided in recovering such effects by deconvolution. The transfer function was obtained by measuring and fitting the system impulse response using single-pole approximation. An iterative deconvolution algorithm was implemented in order to recover the system resolution, while maintaining high signal-to-noise ratio. Results indicated a full recovery of the lidar signal, with resolution matching avalanche photodiodes. Application of such a technique to atmospheric boundary and cloud layers data restores the range resolution, up to 60 m, and overcomes the blurring effects.

  10. Feasibility of using Backscattered Mueller Matrix Images for Bioaerosol Detection

    NASA Astrophysics Data System (ADS)

    Li, Changhui; Kattawar, George W.

    2006-03-01

    It has been shown that by looking at the backscattered radiance from an object illuminated by a laser beam one could effectively distinguish different morphologies from one another. However, if one wants to obtain all the information possible from elastic scattering either from a single particle or an ensemble of particles then one must use the Mueller matrix which contains all the polarization and radiance information available. In this talk, we will show that if we take advantage of the polarization information of the object, many more images related to the overall morphology as well as the internal structure of the object can be obtained. We will present images of the complete Mueller matrix to show the sensitivity of its sixteen components to both external and internal particle properties. We will also show that by using only one or two elements of this matrix one might be able to distinguish bioaerosols such as anthrax from more benign aerosols. We also show that the backscattering Mueller images contain more information than the forward scattering ones.

  11. Laser transmission-backscattering through inhomogeneous cirrus clouds.

    PubMed

    Ou, Szu-Cheng; Takano, Yoshihide; Liou, Kuo-Nan; Lefevre, Randy J; Johnson, Michael W

    2002-09-20

    We have developed a two-dimensional (2D) model for inhomogeneous cirrus clouds in plane-parallel and spherical geometries for the analysis of the transmission and backscattering of high-energy laser beams. The 2D extinction-coefficient and mean effective ice-crystal size fields for cirrus clouds can be determined from a combination of the remote sensing of cirrus clouds by use of the Advanced Very High Resolution Radiometer on board National Oceanic and Atmospheric Administration satellites and the vertical profiling of ice-crystal size distributions available from limited measurements. We demonstrate that satellite remote sensing of the position and the composition of high cirrus can be incorporated directly in the computer model developed for the transmission and backscattering of high-energy laser beams in realistic atmospheres. The results of laser direct transmission, forward scattering, and backscattering are analyzed carefully with respect to aircraft height, cirrus cloud optical depth, and ice-crystal size and orientation. Uncertainty in laser transmission that is due to errors in the retrieved ice-crystal size is negligible. But uncertainty of the order of 2% can be produced if the retrieved optical depth has errors of +/-0.05. With both the aircraft and the target near the cloud top, the direct transmission decreases, owing to the propagation of the laser beam through the curved portion of the cloud top. This effect becomes more pronounced as the horizontal distance between the aircraft and the target increases.

  12. New Examination of the Traditional Raman Lidar Technique II: Evaluating the Ratios for Water Vapor and Aerosols

    NASA Technical Reports Server (NTRS)

    Whiteman, David N.

    2003-01-01

    In a companion paper, the temperature dependence of Raman scattering and its influence on the Raman and Rayleigh-Mie lidar equations was examined. New forms of the lidar equation were developed to account for this temperature sensitivity. Here those results are used to derive the temperature dependent forms of the equations for the water vapor mixing ratio, aerosol scattering ratio, aerosol backscatter coefficient, and extinction to backscatter ratio (Sa). The error equations are developed, the influence of differential transmission is studied and different laser sources are considered in the analysis. The results indicate that the temperature functions become significant when using narrowband detection. Errors of 5% and more can be introduced in the water vapor mixing ratio calculation at high altitudes and errors larger than 10% are possible for calculations of aerosol scattering ratio and thus aerosol backscatter coefficient and extinction to backscatter ratio.

  13. Application of the LIRIC algorithm for the characterization of aerosols during the Airborne Romanian Measurements of Aerosols and Trace gases (AROMAT) campaign

    NASA Astrophysics Data System (ADS)

    Stefanie, Horatiu; Nicolae, Doina; Nemuc, Anca; Belegante, Livio; Toanca, Florica; Ajtai, Nicolae; Ozunu, Alexandru

    2015-04-01

    The ESA/ESTEC AROMAT campaign (Airborne Romanian Measurements of Aerosols and Trace gases) was held between 1st and 14th of September 2014 with the purpose to test and inter-compare newly developed airborne and ground-based instruments dedicated to air quality studies in the context of validation programs of the forthcoming European Space Agency satellites (Sentinel 5P, ADM-Aeolus and EarthCARE). Ground-based remote sensing and airborne in situ measurements were made in southern Romania in order to assess the level and the variability of NO2 and particulate matter, focusing on two areas of interest: SW (Turceni), where many coal based power plants are operating, and SE (Bucharest), affected by intense traffic and partially by industrial pollution. In this paper we present the results obtained after the application of the Lidar - Radiometer Inversion Code (LIRIC) algorithm on combined lidar and sunphotometer data collected at Magurele, 6 km South Bucharest. Full lidar data sets in terms of backscatter signals at 355, 532 and 1064 nm, as well as depolarization at 532 nm were used and combined with Aerosol Robotic Network (AERONET) data, in order to retrieve the profiles of aerosol volume concentrations, separated as fine, spherical and spheroidal coarse modes. Preliminary results showed that aerosols generated by traffic and industrial activities were present in the Planetary Boundary Layer, while biomass burning aerosols transported from the Balkan Peninsula were detected in the upper layers. Acknowledgements: ***This work has been supported by Programme for Research- Space Technology and Advanced Research - STAR, project number 55/2013 - CARESSE. ***The financial support by the European Community's FP7 - PEOPLE 2011 under ITaRS Grant Agreement n° 289923 is gratefully acknowledged.