A Global Modeling Study on Carbonaceous Aerosol Microphysical Characteristics and Radiative Effects

NASA Technical Reports Server (NTRS)

Bauer, S. E.; Menon, S.; Koch, D.; Bond, T. C.; Tsigaridis, K.

2010-01-01

Recently, attention has been drawn towards black carbon aerosols as a short-term climate warming mitigation candidate. However the global and regional impacts of the direct, indirect and semi-direct aerosol effects are highly uncertain, due to the complex nature of aerosol evolution and the way that mixed, aged aerosols interact with clouds and radiation. A detailed aerosol microphysical scheme, MATRIX, embedded within the GISS climate model is used in this study to present a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative effects. Our best estimate for net direct and indirect aerosol radiative flux change between 1750 and 2000 is -0.56 W/m2. However, the direct and indirect aerosol effects are quite sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative flux change can vary between -0.32 to -0.75 W/m2 depending on these carbonaceous particle properties at emission. Taking into account internally mixed black carbon particles let us simulate correct aerosol absorption. Absorption of black carbon aerosols is amplified by sulfate and nitrate coatings and, even more strongly, by organic coatings. Black carbon mitigation scenarios generally showed reduced radiative fluxeswhen sources with a large proportion of black carbon, such as diesel, are reduced; however reducing sources with a larger organic carbon component as well, such as bio-fuels, does not necessarily lead to a reduction in positive radiative flux.

A global modeling study on carbonaceous aerosol microphysical characteristics and radiative effects

NASA Astrophysics Data System (ADS)

Bauer, S. E.; Menon, S.; Koch, D.; Bond, T. C.; Tsigaridis, K.

2010-08-01

Recently, attention has been drawn towards black carbon aerosols as a short-term climate warming mitigation candidate. However the global and regional impacts of the direct, indirect and semi-direct aerosol effects are highly uncertain, due to the complex nature of aerosol evolution and the way that mixed, aged aerosols interact with clouds and radiation. A detailed aerosol microphysical scheme, MATRIX, embedded within the GISS climate model is used in this study to present a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative effects. Our best estimate for net direct and indirect aerosol radiative flux change between 1750 and 2000 is -0.56 W/m2. However, the direct and indirect aerosol effects are quite sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative flux change can vary between -0.32 to -0.75 W/m2 depending on these carbonaceous particle properties at emission. Taking into account internally mixed black carbon particles let us simulate correct aerosol absorption. Absorption of black carbon aerosols is amplified by sulfate and nitrate coatings and, even more strongly, by organic coatings. Black carbon mitigation scenarios generally showed reduced radiative fluxeswhen sources with a large proportion of black carbon, such as diesel, are reduced; however reducing sources with a larger organic carbon component as well, such as bio-fuels, does not necessarily lead to a reduction in positive radiative flux.

Host Model Uncertainty in Aerosol Radiative Effects: the AeroCom Prescribed Experiment and Beyond

NASA Astrophysics Data System (ADS)

Stier, Philip; Schutgens, Nick; Bian, Huisheng; Boucher, Olivier; Chin, Mian; Ghan, Steven; Huneeus, Nicolas; Kinne, Stefan; Lin, Guangxing; Myhre, Gunnar; Penner, Joyce; Randles, Cynthia; Samset, Bjorn; Schulz, Michael; Yu, Hongbin; Zhou, Cheng; Bellouin, Nicolas; Ma, Xiaoyan; Yu, Fangqun; Takemura, Toshihiko

2013-04-01

Anthropogenic and natural aerosol radiative effects are recognized to affect global and regional climate. Multi-model "diversity" in estimates of the aerosol radiative effect is often perceived as a measure of the uncertainty in modelling aerosol itself. However, current aerosol models vary considerably in model components relevant for the calculation of aerosol radiative forcings and feedbacks and the associated "host-model uncertainties" are generally convoluted with the actual uncertainty in aerosol modelling. In the AeroCom Prescribed intercomparison study we systematically isolate and quantify host model uncertainties on aerosol forcing experiments through prescription of identical aerosol radiative properties in eleven participating models. Host model errors in aerosol radiative forcing are largest in regions of uncertain host model components, such as stratocumulus cloud decks or areas with poorly constrained surface albedos, such as sea ice. Our results demonstrate that host model uncertainties are an important component of aerosol forcing uncertainty that require further attention. However, uncertainties in aerosol radiative effects also include short-term and long-term feedback processes that will be systematically explored in future intercomparison studies. Here we will present an overview of the proposals for discussion and results from early scoping studies.

Aerosol Direct Radiative Effects and Heating in the New Era of Active Satellite Observations

NASA Astrophysics Data System (ADS)

Matus, Alexander V.

Atmospheric aerosols impact the global energy budget by scattering and absorbing solar radiation. Despite their impacts, aerosols remain a significant source of uncertainty in our ability to predict future climate. Multi-sensor observations from the A-Train satellite constellation provide valuable observational constraints necessary to reduce uncertainties in model simulations of aerosol direct effects. This study will discuss recent efforts to quantify aerosol direct effects globally and regionally using CloudSat's radiative fluxes and heating rates product. Improving upon previous techniques, this approach leverages the capability of CloudSat and CALIPSO to retrieve vertically resolved estimates of cloud and aerosol properties critical for accurately evaluating the radiative impacts of aerosols. We estimate the global annual mean aerosol direct effect to be -1.9 +/- 0.6 W/m2, which is in better agreement with previously published estimates from global models than previous satellite-based estimates. Detailed comparisons against a fully coupled simulation of the Community Earth System Model, however, reveal that this agreement on the global annual mean masks large regional discrepancies between modeled and observed estimates of aerosol direct effects related to model biases in cloud cover. A low bias in stratocumulus cloud cover over the southeastern Pacific Ocean, for example, leads to an overestimate of the radiative effects of marine aerosols. Stratocumulus clouds over the southeastern Atlantic Ocean can enhance aerosol absorption by 50% allowing aerosol layers to remain self-lofted in an area of subsidence. Aerosol heating is found to peak at 0.6 +/- 0.3 K/day an altitude of 4 km in September when biomass burning reaches a maximum. Finally, the contributions of observed aerosols components are evaluated to estimate the direct radiative forcing of anthropogenic aerosols. Aerosol forcing is computed using satellite-based radiative kernels that describe the

aerosol radiative effects and forcing: spatial and temporal distributions

NASA Astrophysics Data System (ADS)

Kinne, Stefan

2014-05-01

A monthly climatology for aerosol optical properties based on a synthesis from global modeling and observational data has been applied to illustrate spatial distributions and global averages of aerosol radiative impacts. With the help of a pre-industrial reference for aerosol optical properties from global modeling, also the aerosol direct forcing (ca -0.35W/m2 globally and annual averaged) and their spatial and seasonal distributions and contributions by individual aerosol components are estimated. Finally, CCN and IN concentrations associated with this climatology are applied to estimate aerosol indirect effects and forcing.

Estimation of Aerosol Direct Radiative Effects from Satellite and In Situ Measurements

NASA Technical Reports Server (NTRS)

Bergstrom, Robert W.; Russell, Philip B.; Schmid, Beat; Redemann, Jens; McIntosh, Dawn

2000-01-01

Ames researchers have combined measurements from satellite, aircraft, and the surface to estimate the effect of airborne particles (aerosols) on the solar radiation over the North Atlantic region. These aerosols (which come from both natural and pollution sources) can reflect solar radiation, causing a cooling effect that opposes the warming caused by carbon dioxide. Recently, increased attention has been paid to aerosol effects to better understand the Earth climate system.

Indirect effect of changing aerosol concentrations on methane and ozone radiative forcing

NASA Astrophysics Data System (ADS)

Rowlinson, Matthew; Rap, Alexandru; Arnold, Steve; Forster, Piers; Chipperfield, Martyn

2017-04-01

Atmospheric aerosols interact with climate in number of complex ways and quantifying the overall effect remains the dominant uncertainty in estimating anthropogenic climate forcing (IPCC, 2013). The radiative forcing (RF) caused by the direct effect of aerosol interacting with radiation is estimated at -0.35 (-0.85 to +0.15) Wm-2, while cloud-aerosol interactions are estimated at -0.45 (-1.2 to 0.0) Wm-2 (IPCC, 2013). The net impact is a cooling with an effective radiative forcing (ERF) of 0.9 (-1.9 to -0.1) Wm-2 (IPCC, 2013). One effect of aerosols which has not been well evaluated is their effect on atmospheric chemistry. Atmospheric aerosols provide a surface for homogeneous reactions to occur, altering reactions rates and the availability of oxidants, thereby influencing the removal/production of radiatively important species such as methane (CH4) and tropospheric ozone (O3). Oxidants such as the hydroxyl radical (OH) determine the atmospheric lifetime and hence burden of CH4, therefore changes to atmospheric aerosols which impact oxidation chemistry will also influence RF due to CH4. This effect could enhance or offset the negative RF of aerosols, depending on how the individual aerosol changes availability of oxidants. Quantifying the importance of this mechanism for RF is necessary to provide accurate estimates of the effect of aerosols, and assess relative effectiveness of measures to decrease aerosol emissions and precursors. Using a sophisticated aerosol micro-physics model (GLOMAP) coupled to the TOMCAT three-dimensional chemical transport model, we separately simulate changes in atmospheric composition resulting from a 50% decline in anthropogenic emissions of black carbon aerosol (BC), volatile organic compounds (VOCs) and anthropogenic precursors of sulphate and nitrate. The impact of changes to each aerosol on lifetime of CH4 is then calculated to establish the resulting impact on CH4 burden and RF. Cutting global anthropogenic SO2 emissions by 50

Modeling Trends in Tropospheric Aerosol Burden & Its Radiative Effects

EPA Science Inventory

Large changes in emissions of aerosol precursors have occurred across the southeast U.S., North America, as well as the northern hemisphere. The spatial heterogeneity and contrasting trends in the aerosol burden is resulting in differing effects on regional radiative balance. Mul...

Radiative effects of interannually varying vs. interannually invariant aerosol emissions from fires

DOE Office of Scientific and Technical Information (OSTI.GOV)

Grandey, Benjamin S.; Lee, Hsiang-He; Wang, Chien

Open-burning fires play an important role in the earth's climate system. In addition to contributing a substantial fraction of global emissions of carbon dioxide, they are a major source of atmospheric aerosols containing organic carbon, black carbon, and sulfate. These “fire aerosols” can influence the climate via direct and indirect radiative effects. In this study, we investigate these radiative effects and the hydrological fast response using the Community Atmosphere Model version 5 (CAM5). Emissions of fire aerosols exert a global mean net radiative effect of −1.0 W m −2, dominated by the cloud shortwave response to organic carbon aerosol. The net radiative effectmore » is particularly strong over boreal regions. Conventionally, many climate modelling studies have used an interannually invariant monthly climatology of emissions of fire aerosols. However, by comparing simulations using interannually varying emissions vs. interannually invariant emissions, we find that ignoring the interannual variability of the emissions can lead to systematic overestimation of the strength of the net radiative effect of the fire aerosols. Globally, the overestimation is +23 % (−0.2 W m −2). Regionally, the overestimation can be substantially larger. For example, over Australia and New Zealand the overestimation is +58 % (−1.2 W m −2), while over Boreal Asia the overestimation is +43 % (−1.9 W m −2). The systematic overestimation of the net radiative effect of the fire aerosols is likely due to the non-linear influence of aerosols on clouds. However, ignoring interannual variability in the emissions does not appear to significantly impact the hydrological fast response. In order to improve understanding of the climate system, we need to take into account the interannual variability of aerosol emissions.« less

Radiative effects of interannually varying vs. interannually invariant aerosol emissions from fires

DOE PAGES

Grandey, Benjamin S.; Lee, Hsiang-He; Wang, Chien

2016-11-23

Open-burning fires play an important role in the earth's climate system. In addition to contributing a substantial fraction of global emissions of carbon dioxide, they are a major source of atmospheric aerosols containing organic carbon, black carbon, and sulfate. These “fire aerosols” can influence the climate via direct and indirect radiative effects. In this study, we investigate these radiative effects and the hydrological fast response using the Community Atmosphere Model version 5 (CAM5). Emissions of fire aerosols exert a global mean net radiative effect of −1.0 W m −2, dominated by the cloud shortwave response to organic carbon aerosol. The net radiative effectmore » is particularly strong over boreal regions. Conventionally, many climate modelling studies have used an interannually invariant monthly climatology of emissions of fire aerosols. However, by comparing simulations using interannually varying emissions vs. interannually invariant emissions, we find that ignoring the interannual variability of the emissions can lead to systematic overestimation of the strength of the net radiative effect of the fire aerosols. Globally, the overestimation is +23 % (−0.2 W m −2). Regionally, the overestimation can be substantially larger. For example, over Australia and New Zealand the overestimation is +58 % (−1.2 W m −2), while over Boreal Asia the overestimation is +43 % (−1.9 W m −2). The systematic overestimation of the net radiative effect of the fire aerosols is likely due to the non-linear influence of aerosols on clouds. However, ignoring interannual variability in the emissions does not appear to significantly impact the hydrological fast response. In order to improve understanding of the climate system, we need to take into account the interannual variability of aerosol emissions.« less

New approaches to quantifying aerosol influence on the cloud radiative effect.

PubMed

Feingold, Graham; McComiskey, Allison; Yamaguchi, Takanobu; Johnson, Jill S; Carslaw, Kenneth S; Schmidt, K Sebastian

2016-05-24

The topic of cloud radiative forcing associated with the atmospheric aerosol has been the focus of intense scrutiny for decades. The enormity of the problem is reflected in the need to understand aspects such as aerosol composition, optical properties, cloud condensation, and ice nucleation potential, along with the global distribution of these properties, controlled by emissions, transport, transformation, and sinks. Equally daunting is that clouds themselves are complex, turbulent, microphysical entities and, by their very nature, ephemeral and hard to predict. Atmospheric general circulation models represent aerosol-cloud interactions at ever-increasing levels of detail, but these models lack the resolution to represent clouds and aerosol-cloud interactions adequately. There is a dearth of observational constraints on aerosol-cloud interactions. We develop a conceptual approach to systematically constrain the aerosol-cloud radiative effect in shallow clouds through a combination of routine process modeling and satellite and surface-based shortwave radiation measurements. We heed the call to merge Darwinian and Newtonian strategies by balancing microphysical detail with scaling and emergent properties of the aerosol-cloud radiation system.

Aerosol optical properties and radiative effects: Assessment of urban aerosols in central China using 10-year observations

NASA Astrophysics Data System (ADS)

Zhang, Ming; Ma, Yingying; Gong, Wei; Liu, Boming; Shi, Yifan; Chen, ZhongYong

2018-06-01

Poor air quality episodes are common in central China. Here, based on 10 years of ground-based sun-photometric observations, aerosol optical and radiative forcing characteristics were analyzed in Wuhan, the biggest metropolis in central China. Aerosol optical depth (AOD) in the last decade declined significantly, while the Ångström exponent (AE) showed slight growth. Single scattering albedo (SSA) at 440 nm reached the lowest value (0.87) in winter and highest value (0.93) in summer. Aerosol parameters derived from sun-photometric observations were used as input in a radiative transfer model to calculate aerosol radiative forcing (ARF) on the surface in ultraviolet (UV), visible (VIS), near-infrared (NIR), and shortwave (SW) spectra. ARFSW sustained decreases (the absolute values) over the last 10 years. In terms of seasonal variability, due to the increases in multiple scattering effects and attenuation of the transmitted radiation as AOD increased, ARF in summer displayed the largest value (-73.94 W/m2). After eliminating the influence of aerosol loading, the maximum aerosol radiative forcing efficiency in SW range (ARFESW) achieved a value of -64.5 W/m2/AOD in April. The ARFE change in each sub-interval spectrum was related to the change in SSA and effective radius of fine mode particles (Refff), that is, ARFE increased with the decreases in SSA and Refff. The smallest contribution of ARFENIR to ARFESW was 34.11% under strong absorbing and fine particle conditions, and opposite results were found for the VIS range, whose values were always over 51.82%. Finally, due to the serious air pollution and frequency of haze day, aerosol characteristics in haze and clear days were analyzed. The percentage of ARFENIR increased from 35.71% on clear-air days to 37.63% during haze periods, while both the percentage of ARFEUV and ARFENIR in ARFESW kept decreasing. The results of this paper should help us to better understand the effect of aerosols on solar spectral radiation

Multidecadal variations of solar radiation reaching the surface and the role of aerosol direct radiative effects

NASA Astrophysics Data System (ADS)

Chin, M.; Diehl, T. L.; Bian, H.; Yu, H.; Kucsera, T. L.; Wild, M., Sr.; Hakuba, M. Z.; Qian, Y.; Stackhouse, P. W., Jr.; Pinker, R. T.; Zhang, Y.; Kato, S.; Loeb, N. G.; Kinne, S.; Streets, D. G.

2017-12-01

Incoming solar radiation drives the Earth's climate system. Long-term surface observations of the solar radiation reaching the surface (RSFC) have shown decreasing or increasing trends, often referred to as solar "dimming" or "brightening", in many regions of the world in the past several decades. Such long-term variation of RSFC mostly reflects the change of the solar-attenuation components within the atmosphere. Anthropogenic emissions of aerosols and precursor gases have changed significantly in the past decades with 50-80% reduction in North America and Europe but an increase of similar magnitude in East and South Asia since 1980, mirroring the change in RSFC over those regions. This has led to suggestions that aerosols play a critical role in determining RSFC trends. This work is to assess the role of direct radiative effects of aerosols on the solar "dimming" and "brightening" trends with modeling studies. First, we will show the trends of aerosol optical depth (AOD) and aerosol surface concentrations in different regions from 1980 to 2009 with remote sensing and in-situ data as well as model simulations, and attribute those changes to anthropogenic or natural sources. We will then show the trends of RSFC from the model and compare the results with observations from the surface networks and satellite-based products. Furthermore, we will use the GOCART model to attribute the "dimming/ brightening" trends to the changes of aerosols through the direct radiative effects. Finally, we will discuss the way forward to understand the aerosol effects on RSFC (as well as on other climate variables) through aerosol-cloud-radiation interactions.

A Study of Aerosol Direct Radiative Effect and Its Impacts on Global Terrestrial Ecosystem Cycles

NASA Astrophysics Data System (ADS)

Zhang, J.; Shao, S.; Zhou, L.

2017-12-01

Aerosols can absorb and scatter solar radiation, thus cause the total solar radiation reaching the surface to drop and the fraction of diffuse radiation to increase, which influence the surface radiation budget. The global surface radiation with and without consideration of aerosols are calculated by the Fu-Liou atmospheric radiative transfer model based on the MODIS aerosol products, CERES cloud products and other remote sensing data. The aerosol direct radiative effect is calculated based on the two scenarios of aerosols. Our calculation showed that in 2007, aerosols decreased the global total radiation by 9.16 W m-2 on average. Large decrease generally occurred in places with high AOD. As for the diffuse radiation, aerosol-induced changes were either positive or negative. Large increase generally occurred in places with high surface albedo, while large decrease generally occurred in places with high cloud fraction. The global aerosol-induced diffuse radiation change averaged 8.17 W m-2 in 2007. The aerosol direct radiative effect causes the photosynthetic active radiation to increase, and its influences on the global carbon cycle of terrestrial ecosystem are studied by using the Community Land Model (CLM). Calculations show that the aerosol direct radiative effects caused the global averages of terrestrial gross primary productivity (GPP), net primary productivity (NPP), heterotrophic respiration (RH), autotrophic respiration (RA), and net ecosystem productivity (Reco) to increase in 2007, with significant spatial variations however. The global average changes of GPP, NPP, NEP, RA, RH and Reco in 2007 were +6.47 gC m-2, +2.23 gC m-2, +0.34 gC m-2, +4.24 gC m-2, +1.89 gC m-2, +6.13 gC m-2, respectively. Examinations of the carbon fluxes show that the aerosol direct radiative effects influence the terrestrial ecosystem carbon cycles via the following two approaches: First, the diffuse fertilization effect, i.e. more diffuse radiation absorbed by vegetation shade

Radiative Effects of Atmospheric Aerosols and Impacts on Solar Photovoltaic Electricity Generation

NASA Astrophysics Data System (ADS)

Lund, Cory Christopher

Atmospheric aerosols, by scattering and absorbing radiation, perturbs the Earth's energy balance and reduces the amount of insolation reaching the surface. This dissertation first studies the radiative effects of aerosols by analyzing the internal mixing of various aerosol species. It then examines the aerosol impact on solar PV efficiency and the resulting influence on power systems, including both atmospheric aerosols and deposition of particulate matter (PM) on PV surfaces,. Chapter 2 studies the radiative effects of black carbon (BC), sulfate and organic carbon (OC) internal mixing using a simple radiative transfer model. I find that internal mixing may not result in a positive radiative forcing compared to external mixing, but blocks additional shortwave radiation from the surface, enhancing the surface dimming effect. Chapter 3 estimates the impact of atmospheric aerosol attenuation on solar PV resources in China using a PV performance model with satellite-derived long-term surface irradiance data. I find that, in Eastern China, annual average reductions of solar resources due to aerosols are more than 20%, with comparable impacts to clouds in winter. Improving air quality in China would increase efficiency of solar PV generation. As a positive feedback, increased PV efficiency and deployment would further reduce air pollutant emissions too. Chapter 4 further quantifies the total aerosol impact on PV efficiency globally, including both atmospheric aerosols and the deposition of PM on PV surfaces. I find that, if panels are uncleaned and soiling is only removed by precipitation, deposition of PM accounts for more than two-thirds of the total aerosol impact in most regions. Cleaning the panels, even every few months, would largely increase PV efficiency in resource-abundant regions. Chapter 5 takes a further step to evaluate the impact of PV generation reduction due to aerosols on a projected 2030 power system in China with 400GW of PV. I find that aerosols

Climatic Effects of 1950-2050 Changes in US Anthropogenic Aerosols. Part 1; Aerosol Trends and Radiative Forcing

NASA Technical Reports Server (NTRS)

Leibensperger, E. M.; Mickley, L. J.; Jacob, D. J.; Chen, W.-T.; Seinfeld, J. H.; Nenes, A.; Adams, P. J.; Streets, D. G.; Kumar, N.; Rind, D.

2012-01-01

We calculate decadal aerosol direct and indirect (warm cloud) radiative forcings from US anthropogenic sources over the 1950-2050 period. Past and future aerosol distributions are constructed using GEOS-Chem and historical emission inventories and future projections from the IPCC A1B scenario. Aerosol simulations are evaluated with observed spatial distributions and 1980-2010 trends of aerosol concentrations and wet deposition in the contiguous US. Direct and indirect radiative forcing is calculated using the GISS general circulation model and monthly mean aerosol distributions from GEOS-Chem. The radiative forcing from US anthropogenic aerosols is strongly localized over the eastern US. We find that its magnitude peaked in 1970-1990, with values over the eastern US (east of 100 deg W) of -2.0Wm(exp-2 for direct forcing including contributions from sulfate (-2.0Wm-2), nitrate (-0.2Wm(exp-2), organic carbon (-0.2Wm(exp-2), and black carbon (+0.4Wm(exp-2). The uncertainties in radiative forcing due to aerosol radiative properties are estimated to be about 50 %. The aerosol indirect effect is estimated to be of comparable magnitude to the direct forcing. We find that the magnitude of the forcing declined sharply from 1990 to 2010 (by 0.8Wm(exp-2) direct and 1.0Wm(exp-2 indirect), mainly reflecting decreases in SO2 emissions, and project that it will continue declining post-2010 but at a much slower rate since US SO2 emissions have already declined by almost 60% from their peak. This suggests that much of the warming effect of reducing US anthropogenic aerosol sources has already been realized. The small positive radiative forcing from US BC emissions (+0.3Wm(exp-2 over the eastern US in 2010; 5% of the global forcing from anthropogenic BC emissions worldwide) suggests that a US emission control strategy focused on BC would have only limited climate benefit.

Global radiative effects of solid fuel cookstove aerosol emissions

NASA Astrophysics Data System (ADS)

Huang, Yaoxian; Unger, Nadine; Storelvmo, Trude; Harper, Kandice; Zheng, Yiqi; Heyes, Chris

2018-04-01

We apply the NCAR CAM5-Chem global aerosol-climate model to quantify the net global radiative effects of black and organic carbon aerosols from global and Indian solid fuel cookstove emissions for the year 2010. Our assessment accounts for the direct radiative effects, changes to cloud albedo and lifetime (aerosol indirect effect, AIE), impacts on clouds via the vertical temperature profile (semi-direct effect, SDE) and changes in the surface albedo of snow and ice (surface albedo effect). In addition, we provide the first estimate of household solid fuel black carbon emission effects on ice clouds. Anthropogenic emissions are from the IIASA GAINS ECLIPSE V5a inventory. A global dataset of black carbon (BC) and organic aerosol (OA) measurements from surface sites and aerosol optical depth (AOD) from AERONET is used to evaluate the model skill. Compared with observations, the model successfully reproduces the spatial patterns of atmospheric BC and OA concentrations, and agrees with measurements to within a factor of 2. Globally, the simulated AOD agrees well with observations, with a normalized mean bias close to zero. However, the model tends to underestimate AOD over India and China by ˜ 19 ± 4 % but overestimate it over Africa by ˜ 25 ± 11 % (± represents modeled temporal standard deviations for n = 5 run years). Without BC serving as ice nuclei (IN), global and Indian solid fuel cookstove aerosol emissions have net global cooling radiative effects of -141 ± 4 mW m-2 and -12 ± 4 mW m-2, respectively (± represents modeled temporal standard deviations for n = 5 run years). The net radiative impacts are dominated by the AIE and SDE mechanisms, which originate from enhanced cloud condensation nuclei concentrations for the formation of liquid and mixed-phase clouds, and a suppression of convective transport of water vapor from the lower troposphere to the upper troposphere/lower stratosphere that in turn leads to reduced ice cloud formation. When BC is allowed

Aerosol Radiative Effects on Deep Convective Clouds and Associated Radiative Forcing

NASA Technical Reports Server (NTRS)

Fan, J.; Zhang, R.; Tao, W.-K.; Mohr, I.

2007-01-01

The aerosol radiative effects (ARE) on the deep convective clouds are investigated by using a spectral-bin cloud-resolving model (CRM) coupled with a radiation scheme and an explicit land surface model. The sensitivity of cloud properties and the associated radiative forcing to aerosol single-scattering albedo (SSA) are examined. The ARE on cloud properties is pronounced for mid-visible SSA of 0.85. Relative to the case excluding the ARE, cloud fraction and optical depth decrease by about 18% and 20%, respectively. Cloud droplet and ice particle number concentrations, liquid water path (LWP), ice water path (IWP), and droplet size decrease significantly when the ARE is introduced. The ARE causes a surface cooling of about 0.35 K and significantly high heating rates in the lower troposphere (about 0.6K/day higher at 2 km), both of which lead to a more stable atmosphere and hence weaker convection. The weaker convection and the more desiccation of cloud layers explain the less cloudiness, lower cloud optical depth, LWP and IWP, smaller droplet size, and less precipitation. The daytime-mean direct forcing induced by black carbon is about 2.2 W/sq m at the top of atmosphere (TOA) and -17.4 W/sq m at the surface for SSA of 0.85. The semi-direct forcing is positive, about 10 and 11.2 W/sq m at the TOA and surface, respectively. Both the TOA and surface total radiative forcing values are strongly negative for the deep convective clouds, attributed mostly to aerosol indirect forcing. Aerosol direct and semi-direct effects are very sensitive to SSA. Because the positive semi-direct forcing compensates the negative direct forcing at the surface, the surface temperature and heat fluxes decrease less significantly with the increase of aerosol absorption (decreasing SSA). The cloud fraction, optical depth, convective strength, and precipitation decrease with the increase of absorption, resulting from a more stable and dryer atmosphere due to enhanced surface cooling and

Dust aerosol radiative effect and influence on urban atmospheric boundary layer

NASA Astrophysics Data System (ADS)

Zhang, L.; Chen, M.; Li, L.

2007-11-01

An 1.5-level-closure and 3-D non-stationary atmospheric boundary layer (ABL) model and a radiation transfer model with the output of Weather Research and Forecast (WRF) Model and lidar AML-1 are employed to simulate the dust aerosol radiative effect and its influence on ABL in Beijing for the period of 23-26 January 2002 when a dust storm occurred. The simulation shows that daytime dust aerosol radiative effect heats up the ABL at the mean rate of about 0.68 K/h. The horizontal wind speed from ground to 900 m layer is also overall increased, and the value changes about 0.01 m/s at 14:00 LT near the ground. At night, the dust aerosol radiative effect cools the ABL at the mean rate of -0.21 K/h and the wind speed lowers down at about -0.19 m/s at 02:00 LT near the ground.

Internally Consistent MODIS Estimate of Aerosol Clear-Sky Radiative Effect Over the Global Oceans

NASA Technical Reports Server (NTRS)

Remer, Lorraine A.; Kaufman, Yoram J.

2004-01-01

Modern satellite remote sensing, and in particular the MODerate resolution Imaging Spectroradiometer (MODIS), offers a measurement-based pathway to estimate global aerosol radiative effects and aerosol radiative forcing. Over the Oceans, MODIS retrieves the total aerosol optical thickness, but also reports which combination of the 9 different aerosol models was used to obtain the retrieval. Each of the 9 models is characterized by a size distribution and complex refractive index, which through Mie calculations correspond to a unique set of single scattering albedo, assymetry parameter and spectral extinction for each model. The combination of these sets of optical parameters weighted by the optical thickness attributed to each model in the retrieval produces the best fit to the observed radiances at the top of the atmosphere. Thus the MODIS Ocean aerosol retrieval provides us with (1) An observed distribution of global aerosol loading, and (2) An internally-consistent, observed, distribution of aerosol optical models that when used in combination will best represent the radiances at the top of the atmosphere. We use these two observed global distributions to initialize the column climate model by Chou and Suarez to calculate the aerosol radiative effect at top of the atmosphere and the radiative efficiency of the aerosols over the global oceans. We apply the analysis to 3 years of MODIS retrievals from the Terra satellite and produce global and regional, seasonally varying, estimates of aerosol radiative effect over the clear-sky oceans.

Aerosol radiative effects over BIMSTEC regions

NASA Astrophysics Data System (ADS)

Kumar, Sumit; Kar, S. C.; Mupparthy, Raghavendra S.

Aerosols can have variety of shapes, composition, sizes and other properties that influence their optical characteristics and thus the radiative impact. The visible impact of aerosol is the formation of haze, a layer of particles from vehicular, industrial emissions and biomass burning. The characterization of these fine particles is important for regulators and researchers because of their potential impact on human health, their ability to travel thousands of kilometers crossing international borders, and their influence on climate forcing and global warming. The Bay of Bengal Initiative for Multi-Sectoral Technical and Economic Cooperation (BIMSTEC) with Member Countries Bangladesh, Bhutan, India, Myanmar, Nepal, Sri Lanka and Thailand has emerged as an important regional group for technical and economic Cooperation. Continuing the quest for a deeper understanding of BIMSTEC countries weather and climate, in this paper we focused on aerosols and their direct radiative effects. Because of various contrasts like geophysical, agricultural practices, heterogeneous land/ocean surface, population etc these regions present an excellent natural laboratory for studying aerosol-meteorology interactions in tropical to sub-tropical environments. We exploited data available on multiple platforms (such as MISR, MODIS etc) and models (OPAC, SBDART etc) to compute the results. Ten regions were selected with different surface characteristics, also having considerable differences in the long-term trends and seasonal distribution of aerosols. In a preliminary analysis pertaining to pre-monsoon (March-April-May) of 2013, AOD _{555nm} is found to be maximum over Bangladesh (>0.52) and minimum over Bhutan (0.22), whereas other regions have intermediate values. Concurrent to these variability of AOD we found a strong reduction in incoming flux at surface of all the regions (> -25 Wm (-2) ), except Bhutan and Sri Lanka (< -18Wm (-2) ). The top of the atmosphere (TOA) forcing values are

How Models Simulate the Radiative Effect in the Transition Zone of the Aerosol-Cloud Continuum

NASA Astrophysics Data System (ADS)

Calbo Angrill, J.; González, J. A.; Long, C. N.; McComiskey, A. C.

2017-12-01

Several studies have pointed towards dealing with clouds and aerosols as two manifestations of what is essentially the same physical phenomenon: a suspension of tiny particles in the air. Although the two extreme cases (i.e., pure aerosol and well-defined cloud) are easily distinguished, and obviously produce different radiative effects, there are many situations in the transition (or "twilight") zone. In a recent paper [Calbó et al., Atmos. Res. 2017, j.atmosres.2017.06.010], the authors of the current communication estimated that about 10% of time there might be a suspension of particles in the air that is difficult to distinguish as either cloud or aerosol. Radiative transfer models, however, simulate the effect of clouds and aerosols with different modules, routines, or parameterizations. In this study, we apply a sensitivity analysis approach to assess the ability of two radiative transfer models (SBDART and RRTM) in simulating the radiative effect of a suspension of particles with characteristics in the boundary between cloud and aerosol. We simulate this kind of suspension either in "cloud mode" or in "aerosol mode" and setting different values of optical depth, droplet size, water path, aerosol type, cloud height, etc. Irradiances both for solar and infrared bands are studied, both at ground level and at the top of the atmosphere, and all analyses are repeated for different solar zenith angles. We obtain that (a) water clouds and ice clouds have similar radiative effects if they have the same optical depth; (b) the spread of effects regarding different aerosol type/aerosol characteristics is remarkable; (c) radiative effects of an aerosol layer and of a cloud layer are different, even if they have similar optical depth; (d) for a given effect on the diffuse component, the effect on the direct component is usually greater (more extinction of direct beam) by aerosols than by clouds; (e) radiative transfer models are somewhat limited when simulating the

Direct radiative effect due to brownness in organic carbon aerosols generated from biomass combustion

NASA Astrophysics Data System (ADS)

Rathod, T. D.; Sahu, S. K.; Tiwari, M.; Pandit, G. G.

2016-12-01

We report the enhancement in the direct radiative effect due the presence of Brown carbon (BrC) as a part of organic carbon aerosols. The optical properties of organic carbon aerosols generated from pyrolytic combustion of mango tree wood (Magnifera Indica) and dung cake at different temperatures were considered. Mie codes were used to calculate absorption and scattering coefficients coupled with experimentally derived imaginary complex refractive index. The direct radiative effect (DRE) for sampled organic carbon aerosols was estimated using a wavelength dependent radiative transfer equation. The BrC DRE was estimated taking virtually non absorbing organic aerosols as reference. The BrC DRE from wood and dung cake was compared at different combustion temperatures and conditions. The BrC contributed positively to the direct top of the atmosphere radiative effect. Dung cake generated BrC aerosols were found to be strongly light absorbing as compared to BrC from wood combustion. It was noted that radiative effects of BrC from wood depended on its generation temperature and conditions. For BrC aerosols from dung cake such strong dependence was not observed. The average BrC aerosol DRE values were 1.53±0.76 W g-1 and 17.84±6.45 W g-1 for wood and dung cake respectively. The DRE contribution of BrC aerosols came mainly (67-90%) from visible light absorption though they exhibited strong absorption in shorter wavelengths of the UV-visible spectrum.

Sensitivity of aerosol radiative forcing efficiency to the coarse mode contributions across aerosol regimes

NASA Astrophysics Data System (ADS)

McComiskey, A. C.; Telg, H.; Sheridan, P. J.; Kassianov, E.

2017-12-01

The coarse mode contribution to the aerosol radiative effect in a range of clean and turbid aerosol regimes has not been well quantified. While the coarse-mode radiative effect in turbid conditions is generally assumed to be consequential, the effect in clean conditions has likely been underestimated. We survey ground-based in situ measurements of the coarse mode fraction of aerosol optical properties measured around the globe over the past 20 years by the DOE Atmospheric Radiation Measurement Facility and the NOAA Global Monitoring Division. The aerosol forcing efficiency is presented, allowing an evaluation of where the aerosol coarse mode might be climatologically significant.

Radiative Effects of Aerosols Generated from Biomass Burning, Dust Storms, and Forest Fires

NASA Technical Reports Server (NTRS)

Christopher Sundar A.; Vulcan, Donna V.; Welch, Ronald M.

1996-01-01

Atmospheric aerosol particles, both natural and anthropogenic, are important to the earth's radiative balance. They scatter the incoming solar radiation and modify the shortwave reflective properties of clouds by acting as Cloud Condensation Nuclei (CCN). Although it has been recognized that aerosols exert a net cooling influence on climate (Twomey et al. 1984), this effect has received much less attention than the radiative forcings due to clouds and greenhouse gases. The radiative forcing due to aerosols is comparable in magnitude to current anthropogenic greenhouse gas forcing but opposite in sign (Houghton et al. 1990). Atmospheric aerosol particles generated from biomass burning, dust storms and forest fires are important regional climatic variables. A recent study by Penner et al. (1992) proposed that smoke particles from biomass burning may have a significant impact on the global radiation balance. They estimate that about 114 Tg of smoke is produced per year in the tropics through biomass burning. The direct and indirect effects of smoke aerosol due to biomass burning could add up globally to a cooling effect as large as 2 W/sq m. Ackerman and Chung (1992) used model calculations and the Earth Radiation Budget Experiment (ERBE) data to show that in comparison to clear days, the heavy dust loading over the Saudi Arabian peninsula can change the Top of the Atmosphere (TOA) clear sky shortwave and longwave radiant exitance by 40-90 W/sq m and 5-20 W/sq m, respectively. Large particle concentrations produced from these types of events often are found with optical thicknesses greater than one. These aerosol particles are transported across considerable distances from the source (Fraser et al. 1984). and they could perturb the radiative balance significantly. In this study, the regional radiative effects of aerosols produced from biomass burning, dust storms and forest fires are examined using the Advanced Very High Resolution Radiometer (AVHRR) Local Area

CALIPSO-Inferred Aerosol Direct Radiative Effects: Bias Estimates Using Ground-Based Raman Lidars

NASA Technical Reports Server (NTRS)

Thorsen, Tyler; Fu, Qiang

2016-01-01

Observational constraints on the change in the radiative energy budget caused by the presence of aerosols, i.e. the aerosol direct radiative effect (DRE), have recently been made using observations from the Cloud- Aerosol Lidar and Infrared Pathfinder Satellite (CALIPSO). CALIPSO observations have the potential to provide improved global estimates of aerosol DRE compared to passive sensor-derived estimates due to CALIPSO's ability to perform vertically-resolved aerosol retrievals over all surface types and over cloud. In this study we estimate the uncertainties in CALIPSO-inferred aerosol DRE using multiple years of observations from the Atmospheric Radiation Measurement (ARM) program's Raman lidars (RL) at midlatitude and tropical sites. Examined are assumptions about the ratio of extinction-to-backscatter (i.e. the lidar ratio) made by the CALIPSO retrievals, which are needed to retrieve the aerosol extinction profile. The lidar ratio is shown to introduce minimal error in the mean aerosol DRE at the top-of-atmosphere and surface. It is also shown that CALIPSO is unable to detect all radiatively-significant aerosol, resulting in an underestimate in the magnitude of the aerosol DRE by 30-50%. Therefore, global estimates of the aerosol DRE inferred from CALIPSO observations are likely too weak.

CALIPSO-Inferred Aerosol Direct Radiative Effects: Bias Estimates Using Ground-Based Raman Lidars

NASA Technical Reports Server (NTRS)

Thorsen, Tyler; Fu, Qiang

2015-01-01

Observational constraints on the change in the radiative energy budget caused by the presence of aerosols, i.e. the aerosol direct radiative effect (DRE), have recently been made using observations from the Cloud- Aerosol Lidar and Infrared Pathfinder Satellite (CALIPSO). CALIPSO observations have the potential to provide improved global estimates of aerosol DRE compared to passive sensor-derived estimates due to CALIPSO's ability to perform vertically-resolved aerosol retrievals over all surface types and over cloud. In this study we estimate the uncertainties in CALIPSO-inferred aerosol DRE using multiple years of observations from the Atmospheric Radiation Measurement (ARM) program's Raman lidars (RL) at mid-latitude and tropical sites. Examined are assumptions about the ratio of extinction-to-backscatter (i.e. the lidar ratio) made by the CALIPSO retrievals, which are needed to retrieve the aerosol extinction profile. The lidar ratio is shown to introduce minimal error in the mean aerosol DRE at the top-of-atmosphere and surface. It is also shown that CALIPSO is unable to detect all radiatively-significant aerosol, resulting in an underestimate in the magnitude of the aerosol DRE by 30â€"50%. Therefore, global estimates of the aerosol DRE inferred from CALIPSO observations are likely too weak.

Estimates of the Spectral Aerosol Single Sea Scattering Albedo and Aerosol Radiative Effects during SAFARI 2000

NASA Technical Reports Server (NTRS)

Bergstrom, Robert W.; Pilewskie, Peter; Schmid, Beat; Russell, Philip B.

2003-01-01

Using measurements of the spectral solar radiative flux and optical depth for 2 days (24 August and 6 September 2000) during the SAFARI 2000 intensive field experiment and a detailed radiative transfer model, we estimate the spectral single scattering albedo of the aerosol layer. The single scattering albedo is similar on the 2 days even though the optical depth for the aerosol layer was quite different. The aerosol single scattering albedo was between 0.85 and 0.90 at 350 nm, decreasing to 0.6 in the near infrared. The magnitude and decrease with wavelength of the single scattering albedo are consistent with the absorption properties of small black carbon particles. We estimate the uncertainty in the single scattering albedo due to the uncertainty in the measured fractional absorption and optical depths. The uncertainty in the single scattering albedo is significantly less on the high-optical-depth day (6 September) than on the low-optical-depth day (24 August). On the high-optical-depth day, the uncertainty in the single scattering albedo is 0.02 in the midvisible whereas on the low-optical-depth day the uncertainty is 0.08 in the midvisible. On both days, the uncertainty becomes larger in the near infrared. We compute the radiative effect of the aerosol by comparing calculations with and without the aerosol. The effect at the top of the atmosphere (TOA) is to cool the atmosphere by 13 W/sq m on 24 August and 17 W/sq m on 6 September. The effect on the downward flux at the surface is a reduction of 57 W/sq m on 24 August and 200 W/sq m on 6 September. The aerosol effect on the downward flux at the surface is in good agreement with the results reported from the Indian Ocean Experiment (INDOEX).

Modeling the radiative effects of biomass burning aerosols on carbon fluxes in the Amazon region

NASA Astrophysics Data System (ADS)

Moreira, Demerval S.; Longo, Karla M.; Freitas, Saulo R.; Yamasoe, Marcia A.; Mercado, Lina M.; Rosário, Nilton E.; Gloor, Emauel; Viana, Rosane S. M.; Miller, John B.; Gatti, Luciana V.; Wiedemann, Kenia T.; Domingues, Lucas K. G.; Correia, Caio C. S.

2017-12-01

Every year, a dense smoke haze covers a large portion of South America originating from fires in the Amazon Basin and central parts of Brazil during the dry biomass burning season between August and October. Over a large portion of South America, the average aerosol optical depth at 550 nm exceeds 1.0 during the fire season, while the background value during the rainy season is below 0.2. Biomass burning aerosol particles increase scattering and absorption of the incident solar radiation. The regional-scale aerosol layer reduces the amount of solar energy reaching the surface, cools the near-surface air, and increases the diffuse radiation fraction over a large disturbed area of the Amazon rainforest. These factors affect the energy and CO2 fluxes at the surface. In this work, we applied a fully integrated atmospheric model to assess the impact of biomass burning aerosols in CO2 fluxes in the Amazon region during 2010. We address the effects of the attenuation of global solar radiation and the enhancement of the diffuse solar radiation flux inside the vegetation canopy. Our results indicate that biomass burning aerosols led to increases of about 27 % in the gross primary productivity of Amazonia and 10 % in plant respiration as well as a decline in soil respiration of 3 %. Consequently, in our model Amazonia became a net carbon sink; net ecosystem exchange during September 2010 dropped from +101 to -104 TgC when the aerosol effects are considered, mainly due to the aerosol diffuse radiation effect. For the forest biome, our results point to a dominance of the diffuse radiation effect on CO2 fluxes, reaching a balance of 50-50 % between the diffuse and direct aerosol effects for high aerosol loads. For C3 grasses and savanna (cerrado), as expected, the contribution of the diffuse radiation effect is much lower, tending to zero with the increase in aerosol load. Taking all biomes together, our model shows the Amazon during the dry season, in the presence of high

Impact of aerosol vertical distribution on aerosol direct radiative effect and heating rate in the Mediterranean region

NASA Astrophysics Data System (ADS)

Pappas, Vasileios; Hatzianastassiou, Nikolaos; Matsoukas, Christos; Koras Carracca, Mario; Kinne, Stefan; Vardavas, Ilias

2015-04-01

It is now well-established that aerosols cause an overall cooling effect at the surface and a warming effect within the atmosphere. At the top of the atmosphere (TOA), both positive and negative forcing can be found, depending on a number of other factors, such as surface albedo and relative position of clouds and aerosols. Whilst aerosol surface cooling is important due to its relation with surface temperature and other bio-environmental reasons, atmospheric heating is of special interest as well having significant impacts on atmospheric dynamics, such as formation of clouds and subsequent precipitation. The actual position of aerosols and their altitude relative to clouds is of major importance as certain types of aerosol, such as black carbon (BC) above clouds can have a significant impact on planetary albedo. The vertical distribution of aerosols and clouds has recently drawn the attention of the aerosol community, because partially can account for the differences between simulated aerosol radiative forcing with various models, and therefore decrease the level of our uncertainty regarding aerosol forcing, which is one of our priorities set by IPCC. The vertical profiles of aerosol optical and physical properties have been studied by various research groups around the world, following different methodologies and using various indices in order to present the impact of aerosols on radiation on different altitudes above the surface. However, there is still variability between the published results as to the actual effect of aerosols on shortwave radiation and on heating rate within the atmosphere. This study uses vertical information on aerosols from the Max Planck Aerosol Climatology (MAC-v1) global dataset, which is a combination of model output with quality ground-based measurements, in order to provide useful insight into the vertical profile of atmospheric heating for the Mediterranean region. MAC-v1 and the science behind this aerosol dataset have already

North Atlantic Aerosol Properties and Direct Radiative Effects: Key Results from TARFOX and ACE-2

NASA Technical Reports Server (NTRS)

Russell, P. B.; Livingston, J. M.; Schmid, B.; Bergstrom, Robert A.; Hignett, P.; Hobbs, P. V.; Durkee, P. A.

2000-01-01

Aerosol effects on atmospheric radiative fluxes provide a forcing function that can change the climate In potentially significant ways. This aerosol radiative forcing is a major source of uncertainty in understanding the observed climate change of the past century and in predicting future climate. To help reduce this uncertainty, the International Global Atmospheric Chemistry Project (IGAC) has endorsed a series of multiplatform aerosol field campaigns. The Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) and the second Aerosol Characterization Experiment (ACE-2) were the first IGAC campaigns to address the impact of anthropogenic aerosols, Both TARFOX and ACE-2 gathered extensive data sets on aerosol properties and radiative effects, TARFOX focused on the urban-industrial haze plume flowing from the eastern United States over the western Atlantic Ocean, whereas ACE-2 studied aerosols carried over the eastern Atlantic from both European urban/industrial and African mineral sources. These aerosols often have a marked influence on the top-of-atmosphere radiances measured by satellites. Shown there are contours of aerosol optical depth derived from radiances measured by the AVHRR sensor on the NOAA-11 satellite. The contours readily show that aerosols originating in North America, Europe, and Africa impact the radiative properties of air over the North Atlantic. However, the accurate derivation of flux changes, or radiative forcing, from the satellite measured radiances or retrieved optical depths remains a difficult challenge. In this paper we summarize key initial results from TARFOX and, to a lesser extent, ACE-2, with a focus on those results that allow an improved assessment of the flux changes caused by North Atlantic aerosols at middle latitudes.

Radiative Importance of Aerosol-Cloud Interaction

NASA Technical Reports Server (NTRS)

Tsay, Si-Chee

1999-01-01

Aerosol particles are input into the troposphere by biomass burning, among other sources. These aerosol palls cover large expanses of the earth's surface. Aerosols may directly scatter solar radiation back to space, thus increasing the earth's albedo and act to cool the earth's surface and atmosphere. Aerosols also contribute to the earth's energy balance indirectly. Hygroscopic aerosol act as cloud condensation nuclei (CCN) and thus affects cloud properties. In 1977, Twomey theorized that additional available CCN would create smaller but more numerous cloud droplets in a cloud with a given amount of liquid water. This in turn would increase the cloud albedo which would scatter additional radiation back to space and create a similar cooling pattern as the direct aerosol effect. Estimates of the magnitude of the aerosol indirect effect on a global scale range from 0.0 to -4.8 W/sq m. Thus the indirect effect can be of comparable magnitude and opposite in sign to the estimates of global greenhouse gas forcing Aerosol-cloud interaction is not a one-way process. Just as aerosols have an influence on clouds through the cloud microphysics, clouds have an influence on aerosols. Cloud droplets are solutions of liquid water and CCN, now dissolved. When the cloud droplet evaporates it leaves behind an aerosol particle. This new particle does not have to have the same properties as the original CCN. In fact, studies show that aerosol particles that result from cloud processing are larger in size than the original CCN. Optical properties of aerosol particles are dependent on the size of the particles. Larger particles have a smaller backscattering fraction, and thus less incoming solar radiation will be backscattered to space if the aerosol particles are larger. Therefore, we see that aerosols and clouds modify each other to influence the radiative balance of the earth. Understanding and quantifying the spatial and seasonal patterns of the aerosol indirect forcing may have

War Induced Aerosol Optical, Microphysical and Radiative Effects

NASA Astrophysics Data System (ADS)

Munshi, Pavel; Tiwari, Shubhansh

2017-01-01

The effect of war on air pollution and climate is assessed in this communication. War today in respect of civil wars and armed conflict in the Middle East area is taken into consideration. Impacts of war are not only in loss of human life and property, but also in the environment. It is well known that war effects air pollution and in the long run contribute to anthropogenic climate change, but general studies on this subject are few because of the difficulties of observations involved. In the current scenario of the ongoing conflict in the Middle East regions, deductions in parameters of atmosphere are discussed. Aerosol Optical Depth, Aerosol loads, Black Carbon, Ozone,Dust, regional haze and many more are analyzed using various satellite data. Multi-model analysis is also studied to verify the analysis. Type segregation of aerosols, in-depth constraints to atmospheric chemistry, biological effects and particularly atmospheric physics in terms of radiative forcing, etc. are discussed. Undergraduate in Earth Sciences.

The direct effect of aerosols on solar radiation over the broader Mediterranean basin

NASA Astrophysics Data System (ADS)

Papadimas, C. D.; Hatzianastassiou, N.; Matsoukas, C.; Kanakidou, M.; Mihalopoulos, N.; Vardavas, I.

2012-08-01

For the first time, the direct radiative effect (DRE) of aerosols on solar radiation is computed over the entire Mediterranean basin, one of the most climatically sensitive world regions, using a deterministic spectral radiation transfer model (RTM). The DRE effects on the outgoing shortwave radiation at the top of atmosphere (TOA), DRETOA, on the absorption of solar radiation in the atmospheric column, DREatm, and on the downward and absorbed surface solar radiation (SSR), DREsurf and DREnetsurf, respectively, are computed separately. The model uses input data for the period 2000-2007 for various surface and atmospheric parameters, taken from satellite (International Satellite Cloud Climatology Project, ISCCP-D2), Global Reanalysis projects (National Centers for Environmental Prediction - National Center for Atmospheric Research, NCEP/NCAR), and other global databases. The spectral aerosol optical properties (aerosol optical depth, AOD, asymmetry parameter, gaer and single scattering albedo, ωaer), are taken from the MODerate resolution Imaging Spectroradiometer (MODIS) of NASA (National Aeronautics and Space Administration) and they are supplemented by the Global Aerosol Data Set (GADS). The model SSR fluxes have been successfully validated against measurements from 80 surface stations of the Global Energy Balance Archive (GEBA) covering the period 2000-2007. A planetary cooling is found above the Mediterranean on an annual basis (regional mean DRETOA = -2.4 W m-2). Although a planetary cooling is found over most of the region, of up to -7 W m-2, large positive DRETOA values (up to +25 W m-2) are found over North Africa, indicating a strong planetary warming, and a weaker warming over the Alps (+0.5 W m-2). Aerosols are found to increase the absorption of solar radiation in the atmospheric column over the region (DREatm = +11.1 W m-2) and to decrease SSR (DREsurf = -16.5 W m-2 and DREnetsurf-13.5 W m-2) inducing thus significant atmospheric warming and surface

Sensitivity of inorganic aerosol radiative effects to U.S. emissions

NASA Astrophysics Data System (ADS)

Holt, J. I.; Solomon, S.; Selin, N. E.

2017-06-01

Between 2005 and 2012, U.S. emissions of nitrogen oxides (NOx) and sulfur dioxide (SO2) decreased by 42% and 62%, respectively. These species, as well as ammonia (NH3), are precursors of inorganic fine aerosols, which scatter incoming shortwave radiation and thus affect climate. Scaling aerosol concentrations to emissions, as might be done for near-term climate projections, neglects nonlinear chemical interactions. To estimate the magnitude of these nonlinearities, we conduct a suite of simulations with a chemical transport model and an off-line radiative transfer model. We find that the direct radiative effect (DRE) over the North American domain decreases by 59 and 160 mW m-2 in winter and summer, respectively, between 2005 and 2012. The sensitivities of DRE to NOx and SO2 emissions increase, by 11% and 21% in summer, while sensitivity to NH3 emissions decreases. The wintertime sensitivity of DRE to NOx emissions is small in 2005 but is 5 times as large in 2012. Scaling radiative effects from 2005 to 2012 based on 2005 sensitivities overestimates the magnitude of the DRE of 7% and 6% of the U.S. attributable DRE in January and July, respectively. The difference between the changes in DRE and the changes in sensitivity suggests that scaling to SO2 emissions alone has so far been an accurate approximation, but it may not be in the near future. These values represent the level of accuracy that can be expected in adjusting aerosol radiative effects in climate models without chemistry.

Radiative Effects of Aerosols

NASA Technical Reports Server (NTRS)

Valero, Francisco P. J.

1996-01-01

During the Atlantic Stratocumulus Transition Experiment (ASTEX) in June 1992, two descents in cloud-free regions allowed comparison of the change in aerosol optical depth as determined by an onboard total-direct-diffuse radiometer (TDDR) to the change calculated from measured size-resolved aerosol microphysics and chemistry. Both profiles included a pollution haze from Europe but the second also included the effect of a Saharan dust layer above the haze. The separate contributions of supermicrometer (coarse) and submicrometer (fine) aerosol were determined and thermal analysis of the pollution haze indicated that the fine aerosol was composed primarily of a sulfate/water mixture with a refractory soot-like core. The soot core increased the calculated extinction by about 10% in the most polluted drier layer relative to a pure sulfate aerosol but had significantly less effect at higher humidities. A 3 km descent through a boundary layer air mass dominated by pollutant aerosol with relative humidities (RH) 10-77% yielded a close agreement between the measured and calculated aerosol optical depths (550 nm) of 0.160 (+/- 0.07) and 0. 157 (+/- 0.034) respectively. During descent the aerosol mass scattering coefficient per unit sulfate mass varied from about 5 to 16 m(exp 2)/g and primarily dependent upon ambient RH. However, the total scattering coefficient per total fine mass was far less variable at about 4+/- 0.7 m(exp 2)/g. A subsequent descent through a Saharan dust layer located above the pollution aerosol layer revealed that both layers contributed similarly to aerosol optical depth. The scattering per unit mass of the coarse aged dust was estimated at 1.1 +/- 0.2 m(exp 2)/g. The large difference (50%) in measured and calculated optical depth for the dust layer exceeded measurements.

Direct radiative effects of aerosols over South Asia from observations and modeling

NASA Astrophysics Data System (ADS)

Nair, Vijayakumar S.; Babu, S. Suresh; Manoj, M. R.; Moorthy, K. Krishna; Chin, Mian

2017-08-01

Quantitative assessment of the seasonal variations in the direct radiative effect (DRE) of composite aerosols as well as the constituent species over the Indian sub continent has been carried out using a synergy of observations from a dense network of ground based aerosol observatories and modeling based on chemical transport model simulations. Seasonal variation of aerosol constituents depict significant influence of anthropogenic aerosol sources in winter and the dominance of natural sources in spring, even though the aerosol optical depth doesn't change significantly between these two seasons. A significant increase in the surface cooling and atmospheric warming has been observed as season changes from winter (DRESUR = -28 ± 12 W m-2 and DREATM = +19.6 ± 9 W m-2) to spring (DRESUR = -33.7 ± 12 W m-2 and DREATM = +27 ± 9 W m-2). Interestingly, springtime aerosols are more absorptive in nature compared to winter and consequently the aerosol induced diabatic heating of the atmosphere goes as high as 1 K day-1 during spring, especially over eastern India. The atmospheric DRE due to dust aerosols (+14 ± 7 W m-2) during spring overwhelms that of black carbon DRE (+11.8 ± 6 W m-2) during winter. The DRE at the top of the atmosphere is mostly governed by the anthropogenic aerosols during all the seasons. The columnar aerosol loading, its anthropogenic fraction and radiative effects shows a steady increase with latitude across Indian mainland leading to a larger aerosol-induced atmospheric warming during spring than in winter.

Aerosol Climate Effects: Local Radiative Forcing and Column Closure Experiments

NASA Technical Reports Server (NTRS)

Russell, P. B.; Bergstrom, Robert W.; Kinne, S. A.

2000-01-01

In an effort to reduce uncertainties in climate change predictions, experiments are being planned and conducted to measure anthropogenic aerosol properties and effects, including effects on radiative fields. The global average, direct anthropogenic aerosol effect on upwelling shortwave fluxes is estimated to be about +1/2 W/sq m, whereas errors in flux changes measured with airborne and spaceborne radiometers are 2 to 8 W/sq m or larger. This poses the question of whether flux changes expected in field experiments will be large enough to measure accurately. This paper obtains a new expression for the aerosol-induced change in upwelling flux, compares it to two-stream and adding-doubling (AD) results, and uses all three methods to estimate expected flux changes. The new expression accounts for the solar zenith angle dependences of aerosol transmission and reflection, as well as of surface albedo, all of which can have a strong effect in determining flux changes measured in field experiments. Despite its relative simplicity, the new expression gives results similar to previous two-stream results. Relative to AD results, it agrees within a few watts per square meter for the intermediate solar elevation angles where the flux changes peak (roughly 10 to 30 degrees), but it has negative errors for higher Sun and positive errors for lower Sun. All three techniques yield aerosol-induced changes in upwelling flux of +8 to +50 W/sq m for aerosol midvisible optical depths of 0.1 to 0.5. Because such aerosol optical depths occur frequently off the U.S. and European Atlantic coasts in summer, the flux changes they induce should be measurable by airborne, and possibly by spaceborne, radiometers, provided sufficient care is taken in experiment design (including measurements to separate aerosol radiative effects from those of absorbing gases). The expected flux changes are about 15 to 100 times larger than the global average flux change expected for the global average

Direct Aerosol Radiative Effects and Heating Rates: Results from the 2016 and 2017 ORACLES Field Campaigns

NASA Astrophysics Data System (ADS)

Cochrane, S.; Schmidt, S.; Chen, H.; Pilewskie, P.; Redemann, J.; LeBlanc, S. E.; Platnick, S. E.; Meyer, K.; Ferrare, R. A.; Burton, S. P.; Hostetler, C. A.; Iwabuchi, H.

2017-12-01

The Southeast Atlantic contains a large, semi-permanent cloud deck often overlaid by a thick layer of biomass burning aerosols that has been advected westward from Southern Africa. We will present (a) the direct aerosol radiative effect (b) the albedo value for which the radiative effect transitions from warming to cooling, i.e., the critical albedo, and (c) aerosol and gas absorption and heating rates for this region from the 2016 and 2017 deployments of the NASA ORACLES experiment (ObseRvations of CLouds above Aerosols and their intEractionS). Observations by the Solar Spectral Flux Radiometer (SSFR), Enhanced MODIS Airborne Simulator (eMAS), High Spectral Resolution Lidar (HSRL-2,) and the Spectrometer for Sky-Scanning Sun-Tracking Atmospheric Research (4STAR) are put into context by the 3D radiative transfer model Monte Carlo Atmospheric Radiative Transfer Simulator (MCARaTS), which allows us to determine the aerosol radiative effect especially when inhomogeneous clouds are present. For highly homogeneous scenes, a direct derivation from the measurements is also possible. We give an overview of spectral single scattering albedo, Ångström exponents, and heating rate profiles for the two experiments while also exploring the dependence of the critical albedo on the aerosol properties.

Modeling Trends in Aerosol Direct Radiative Effects over the Northern Hemisphere using a Coupled Meteorology-Chemistry Model

NASA Astrophysics Data System (ADS)

Mathur, R.; Pleim, J.; Wong, D.; Hogrefe, C.; Xing, J.; Wei, C.; Gan, M.

2013-12-01

While aerosol radiative effects have been recognized as some of the largest sources of uncertainty among the forcers of climate change, the verification of the spatial and temporal variability of the magnitude and directionality of aerosol radiative forcing has remained challenging. A detailed investigation of the processes regulating aerosol distributions, their optical properties, and their radiative effects and verification of their simulated effects for past conditions relative to measurements is needed in order to build confidence in the estimates of the projected impacts arising from changes in both anthropogenic forcing and climate change. Anthropogenic emissions of primary aerosol and gaseous precursors have witnessed dramatic changes over the past two decades across the northern hemisphere. During the period 1990-2010, SO2 and NOx emissions across the US have reduced by about 66% and 50%, respectively, mainly due to Title IV of the U.S. Clean Air Act Amendments (CAA). In contrast, anthropogenic emissions have increased dramatically in many developing regions during this period. We conduct a systematic investigation of changes in anthropogenic emissions of primary aerosols and gaseous precursors over the past two decades, their impacts on trends and spatial heterogeneity in anthropogenic aerosol loading across the northern hemisphere troposphere, and subsequent impacts on regional radiation budgets. The coupled WRF-CMAQ model is applied for selected time periods spanning the period 1990-2010 over a domain covering the northern hemisphere and a nested finer resolution continental U.S. domain. The model includes detailed treatment of direct effects of aerosols on photolysis rates as well as on shortwave radiation. Additionally, treatment of aerosol indirect effects on clouds has also recently been implemented. A methodology is developed to consistently estimate U.S. emission inventories for the 20-year period accounting for air quality regulations as well as

Aerosol Effects on Radiation and Climate: Column Closure Experiments with Towers, Aircraft, and Satellites

NASA Technical Reports Server (NTRS)

Russell, Philip B.

1994-01-01

Many theoretical studies have shown that anthropogenic aerosol particles can change the radiation balance in an atmospheric column and might thereby exert a significant effect on the Earth's climate. In particular, recent calculations have shown that sulfate particles from anthropogenic combustion may already exert a cooling influence on the Earth that partially offsets the warming caused by the greenhouse gases from the same combustion. Despite the potential climatic importance of anthropogenic aerosols, simultaneous measurements of anthropogenic aerosol properties and their effect on atmospheric radiation have been very rare. Successful comparisons of measured radiation fields with those calculated from aerosol measurements - now referred to as column closure comparisons - are required to improve the accuracy and credibility of climate predictions. This paper reviews the column closure experiment performed at the Mt. Sutro Tower in San Francisco in 1975, in which elevated radiometers measured the change in Earth-plus-atmosphere albedo caused by an aerosol layer, while a lidar, sunphotometer, nephelometer, and other radiometers measured properties of the responsible aerosol. The time-dependent albedo calculated from the measured aerosol properties agreed with that measured by the tower radiometers. Also presented are designs for future column closure studies using radiometers and aerosol instruments on the ground, aircraft, and satellites. These designs draw upon algorithms and experience developed in the Sutro Tower study, as well as more recent experience with current measurement and analysis capabilities.

Global Aerosol Radiative Forcing Derived from Sea WiFS-Inferred Aerosol Optical Properties

NASA Technical Reports Server (NTRS)

Chou, Ming-Dah; Chan, Pui-King; Wang, Menghua

1999-01-01

Aerosol optical properties inferred from the Sea-viewing Wide Field-of-view Sensor (SeaWiFS) radiance measurements are used to compute the aerosol shortwave radiative forcing using a radiative transfer model. The aerosol optical thickness at the wavelength of 865-nm is taken from the SeaWIFS archive. It is found that the nominal optical thickness over oceans ranges from 0.1 to 0.2. Using a maritime aerosol model and the radiances measured at the various SeaWiFS channels, the Angstrom exponent is determined to be 0.2174, the single-scattering albedo to be 0.995, and the asymmetry factor to be 0.786. The radiative transfer model has eight bands in the visible and ultraviolet spectral regions and three bands in the near infrared. It includes the absorption due to aerosols, water vapor, carbon dioxide, and oxygen, and the scattering due to aerosols and gases (Rayleigh scattering). The radiative forcing is computed over global oceans for four months (January, April, July, and October, 1998) to represent four seasons. It is found that the aerosol radiative forcing is large and changes significantly with seasons near the continents with large-scale forest fires and desert dust. Averaged over oceans and the four months, the aerosol radiative forcing is approximately 7 W/sq m at the top of the atmosphere. This large radiative forcing is expected to have a significant cooling effect on the Earth's climate as implied from simulations of a number of general circulation models.

Direct Radiative Effects of Aerosols Over South Asia From Observations and Modeling

NASA Technical Reports Server (NTRS)

Nair, Vijayakumar S.; Babu, S. Suresh; Manoj, M. R.; Moorthy, Krishna K.; Chin, Mian

2016-01-01

Quantitative assessment of the seasonal variations in the direct radiative effect (DRE) of composite aerosols as well as the constituent species over the Indian sub continent has been carried out using a synergy of observations from a dense network of ground based aerosol observatories and modeling based on chemical transport model simulations. Seasonal variation of aerosol constituents depict significant influence of anthropogenic aerosol sources in winter and the dominance of natural sources in spring, even though the aerosol optical depth doesn't change significantly between these two seasons. A significant increase in the surface cooling and atmospheric warming has been observed as season changes from winter DRE(sub SUR) = -28 +/- 12 W m(exp -2) and DRE(sub ATM) = +19.6 +/- 9 W m(exp -2) to spring DRE(sub SUR) = -33.7 +/- 12 W m(exp -2) and DRE(sub ATM) = +27 +/- 9 W m(exp-2). Interestingly, springtime aerosols are more absorptive in nature compared to winter and consequently the aerosol induced diabatic heating of the atmosphere goes as high as approximately 1 K day(exp -1) during spring, especially over eastern India. The atmospheric DRE due to dust aerosols (+14 +/- 7 W m(exp 2) during spring overwhelms that of black carbon DRE (+11.8 +/- 6 W m(exp -2) during winter. The DRE at the top of the atmosphere is mostly governed by the anthropogenic aerosols during all the seasons. The columnar aerosol loading, its anthropogenic fraction and radiative effects shows a steady increase with latitude across Indian mainland leading to a larger aerosol-induced atmospheric warming during spring than in winter.

Direct and semidirect aerosol effects of southern African biomass burning aerosol

NASA Astrophysics Data System (ADS)

Sakaeda, Naoko; Wood, Robert; Rasch, Philip J.

2011-06-01

Direct and semidirect radiative effects of biomass burning aerosols from southern African fires during July-October are investigated using 20 year runs of the Community Atmospheric Model (CAM) coupled to a slab ocean model. Aerosol optical depth is constrained using observations in clear skies from Moderate Resolution Imaging Spectroradiometer (MODIS) and for aerosol layers above clouds from Cloud Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO). Over the ocean, where the aerosol layers are primarily located above cloud, negative top of atmosphere (TOA) semidirect radiative effects associated with increased low cloud cover dominate over a weaker positive all-sky direct radiative effect (DRE). In contrast, over the land where the aerosols are often below or within cloud layers, reductions in cloud liquid water path (LWP) lead to a positive semidirect radiative effect that dominates over a near-zero DRE. Over the ocean, the cloud response can be understood as a response to increased lower tropospheric stability (LTS) which is caused both by radiative heating in overlying layers and surface cooling in response to direct aerosol forcing. The marine cloud changes are robust to changes in the cloud parameterization (removal of the hard-wired dependence of clouds on LTS), suggesting that they are physically realistic. Over land, decreased LWP is consistent with weaker convection driven by increased static stability. Over the entire region the overall TOA radiative effect from the biomass burning aerosols is almost zero due to opposing effects over the land and ocean. However, the surface forcing is strongly negative, which leads to a reduction in precipitation and also a reduction in sensible heat flux. The former is primarily realized through reductions in convective precipitation on both the southern and northern flanks of the convective precipitation region spanning the equatorial rain forest and the Intertropical Convergence Zone (ITCZ) in the

Response of different regional online coupled models to aerosol-radiation interactions

NASA Astrophysics Data System (ADS)

Forkel, Renate; Balzarini, Alessandra; Brunner, Dominik; Baró, Rocio; Curci, Gabriele; Hirtl, Marcus; Honzak, Luka; Jiménez-Guerrero, Pedro; Jorba, Oriol; Pérez, Juan L.; Pirovano, Guido; San José, Roberto; Schröder, Wolfram; Tuccella, Paolo; Werhahn, Johannes; Wolke, Ralf; Žabkar, Rahela

2016-04-01

The importance of aerosol-meteorology interactions and their representation in online coupled regional atmospheric chemistry-meteorology models was investigated in COST Action ES1004 (EuMetChem, http://eumetchem.info/). Case study results from different models (COSMO-Muscat, COSMO-ART, and different configurations of WRF-Chem), which were applied for Europe as a coordinated exercise for the year 2010, are analyzed with respect to inter-model variability and the response of the different models to direct and indirect aerosol-radiation interactions. The main focus was on two episodes - the Russian heat wave and wildfires episode in July/August 2010 and a period in October 2010 with enhanced cloud cover and rain and including an of Saharan dust transport to Europe. Looking at physical plausibility the decrease in downward solar radiation and daytime temperature due to the direct aerosol effect is robust for all model configurations. The same holds for the pronounced decrease in cloud water content and increase in solar radiation for cloudy conditions and very low aerosol concentrations that was found for WRF-Chem when aerosol cloud interactions were considered. However, when the differences were tested for statistical significance no significant differences in mean solar radiation and mean temperature between the baseline case and the simulations including the direct and indirect effect from simulated aerosol concentrations were found over Europe for the October episode. Also for the fire episode differences between mean temperature and radiation from the simulations with and without the direct aerosol effect were not significant for the major part of the modelling domain. Only for the region with high fire emissions in Russia, the differences in mean solar radiation and temperature due to the direct effect were found to be significant during the second half of the fire episode - however only for a significance level of 0.1. The few observational data indicate that

An Overview of the Tropospheric Aerosol Radiative Forcing Observational Experiment

NASA Technical Reports Server (NTRS)

Russell, P. B.; Chan, K. Roland (Technical Monitor)

1997-01-01

Aerosol effects on atmospheric radiation are a leading source of uncertainty in predicting future climate. As a result, the International Global Atmospheric Chemistry Program has established a Focus on Atmospheric Aerosols (IGAC/FAA) and endorsed a series of aerosol field campaigns. TARFOX, the second in the IGAC/FAA series, was designed to reduce this uncertainty by measuring aerosol properties and effects in the US eastern seaboard, where one of the world's major plumes of industrial haze moves from the continent over the Atlantic Ocean. TARFOX's objectives are to: 1. Make simultaneous measurements of: (a) aerosol effects on radiation fields, and (b) the chemical, physical, and optical properties of the aerosols causing those effects. 2. Perform a variety of closure studies by using overdetermined data sets to test the mutual consistency of measurements and calculations of a wide range of aerosol properties and effects. 3. Use the results of the closure studies to assess and reduce uncertainties in estimates of aerosol radiative forcing, as well as to guide future field programs. An important subset of the closure studies is tests and improvements of algorithms used to derive aerosol properties and radiative effects from satellite measurements. The TARFOX Intensive Field Period (IFP) was conducted July 10-31, 1996. It included coordinated measurements from four satellites (GOES-8, NOAA-14, ERS-2, LANDSAT), four aircraft (ER-2, C-130, C-131, and a modified Cessna), land sites, and ships. A variety of aerosol conditions was sampled, ranging from relatively clean behind frontal passages to moderately polluted with aerosol optical depths exceeding 0.5 at mid-visible wavelengths. The latter conditions included separate incidents of enhancements caused primarily by anthropogenic sources and another incident of enhancement apparently influenced by recent fog processing. Spatial gradients of aerosol optical thickness were sampled to aid in isolating aerosol effects from

On the Feasibility of Studying Shortwave Aerosol Radiative Forcing of Climate Using Dual-Wavelength Aerosol Backscatter Lidar

NASA Technical Reports Server (NTRS)

Redemann, Jens; Russell, Philip B.; Winker, David M.; McCormick, M. Patrick; Hipskind, R. Stephen (Technical Monitor)

2000-01-01

The current low confidence in the estimates of aerosol-induced perturbations of Earth's radiation balance is caused by the highly non-uniform compositional, spatial and temporal distributions of tropospheric aerosols on a global scale owing to their heterogeneous sources and short lifetimes. Nevertheless, recent studies have shown that the inclusion of aerosol effects in climate model calculations can improve agreement with observed spatial and temporal temperature distributions. In light of the short lifetimes of aerosols, determination of their global distribution with space-borne sensors seems to be a necessary approach. Until recently, satellite measurements of tropospheric aerosols have been approximate and did not provide the full set of information required to determine their radiative effects. With the advent of active aerosol remote sensing from space (e.g., PICASSO-CENA), the applicability fo lidar-derived aerosol 180 deg -backscatter data to radiative flux calculations and hence studies of aerosol effects on climate needs to be investigated.

Carbonaceous Aerosols and Radiative Effects Study (CARES), g1-aircraft, sedlacek sp2

DOE Data Explorer

Sedlacek, Art

2011-08-30

The primary objective of the Carbonaceous Aerosol and Radiative Effects Study (CARES) in 2010 was to investigate the evolution of carbonaceous aerosols of different types and their optical and hygroscopic properties in central California, with a focus on the Sacramento urban plume.

Direct Radiative Effect of Aerosols Based on PARASOL and OMI Satellite Observations

NASA Technical Reports Server (NTRS)

Lacagnina, Carlo; Hasekamp, Otto P.; Torres, Omar

2017-01-01

Accurate portrayal of the aerosol characteristics is crucial to determine aerosol contribution to the Earth's radiation budget. We employ novel satellite retrievals to make a new measurement-based estimate of the shortwave direct radiative effect of aerosols (DREA), both over land and ocean. Global satellite measurements of aerosol optical depth, single-scattering albedo (SSA), and phase function from PARASOL (Polarization and Anisotropy of Reflectances for Atmospheric Sciences coupled with Observations from a Lidar) are used in synergy with OMI (Ozone Monitoring Instrument) SSA. Aerosol information is combined with land-surface bidirectional reflectance distribution function and cloud characteristics from MODIS (Moderate Resolution Imaging Spectroradiometer) satellite products. Eventual gaps in observations are filled with the state-of-the-art global aerosol model ECHAM5-HAM2. It is found that our estimate of DREA is largely insensitive to model choice. Radiative transfer calculations show that DREA at top-of-atmosphere is -4.6 +/- 1.5 W/sq m for cloud-free and -2.1 +/- 0.7 W/sq m for all-sky conditions, during year 2006. These fluxes are consistent with, albeit generally less negative over ocean than, former assessments. Unlike previous studies, our estimate is constrained by retrievals of global coverage SSA, which may justify different DREA values. Remarkable consistency is found in comparison with DREA based on CERES (Clouds and the Earth's Radiant Energy System) and MODIS observations.

Radiative Effects of Aerosol in the Marine Environment: Tales from the Two-Column Aerosol Project

NASA Astrophysics Data System (ADS)

Berg, L. K.; Fast, J. D.; Barnard, J.; Chand, D.; Chapman, E. G.; Comstock, J. M.; Ferrare, R. A.; Flynn, C. J.; Hair, J. W.; Hostetler, C. A.; Hubbe, J.; Johnson, R.; Kassianov, E.; Kluzek, C.; Laskin, A.; Lee, Y.; Mei, F.; Michalsky, J. J.; Redemann, J.; Rogers, R. R.; Russell, P. B.; Sedlacek, A. J.; Schmid, B.; Shilling, J. E.; Shinozuka, Y.; Springston, S. R.; Tomlinson, J. M.; Wilson, J. M.; Zelenyuk, A.; Berkowitz, C. M.

2013-12-01

There is still uncertainty associated with the direct radiative forcing by atmospheric aerosol and its representation in atmospheric models. This is particularly true in marine environments near the coast where the aerosol loading is a function of both naturally occurring and anthropogenic aerosol. These regions are also subject to variable synoptic and thermally driven flows (land-sea breezes) that transport aerosol between the continental and marine environments. The situation is made more complicated due to seasonal changes in aerosol emissions. Given these differences in emissions, we expect significant differences in the aerosol intensive and extensive properties between summer and winter and data is needed to evaluate models over the wide range of conditions. To address this issue, the recently completed Two Column Aerosol Project (TCAP) was designed to measure the key aerosol parameters in two atmospheric columns, one located over Cape Cod, Massachusetts and another approximately 200 km from the coast over the Atlantic Ocean. Measurements included aerosol size distribution, chemical composition, optical properties and vertical distribution. Several aspects make TCAP unique, including the year-long deployment of a suite of surface-based instruments by the US Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility and two aircraft intensive operations periods supported by the ARM Airborne Facility, one conducted in July 2012 and a second in February 2013. The presentation will include a discussion of the impact of the aerosol optical properties and their uncertainty on simulations of the radiation budget within the TCAP domain in the context of both single column and regional scale models. Data from TCAP will be used to highlight a number of important factors, including diurnal variation in aerosol optical depth measured at the surface site, systematic changes in aerosol optical properties (including scattering, absorption, and

Aerosol optical properties and radiative effect under different weather conditions in Harbin, China

NASA Astrophysics Data System (ADS)

Mao, Qianjun; Huang, Chunlin; Zhang, Hengxing; Chen, Qixiang; Yuan, Yuan

2018-03-01

The aerosol optical properties and radiative effect under different weather conditions in Harbin (126.63°E, 45.75°N) were analyzed based on ground-based Sun/Sky radiometric (CE-318) measurements during September 2016-April 2017. The means values of aerosol optical depth (AOD500) and Angstrom exponent (AE440-870) were 0.37 ± 0.27 and 1.08 ± 0.33, respectively. The mean AOD500 under four weather conditions are apparently higher in severe pollution (Se-Po) days (0.80 ± 0.31) and moderate pollution (Mo-Po) days (0.53 ± 0.25) but lower in slight pollution (Sl-Po) days (0.37 ± 0.26) and no pollution (No-Po) days (0.26 ± 0.20), while the mean values of AE440-870 maintain high, varying from 0.98 to 1.25. The higher AE440-870 indicated that the air quality in Harbin is mainly affected by aerosols originated from anthropogenic sources. The daily values of shortwave (0.25-4 μm) direct aerosol radiative forcing (DARF) at top/bottom of atmosphere (TOA/BOA) were estimated through Santa Barbara DISORT Atmosphere Radiative Transfer (SBDART) model. Further, the aerosol radiative forcing efficiency (ARFE), radiation flux (RF) and atmosphere heating rate (HR) in Harbin were also estimated by the SBDART model.

Experimental Characterization of Radiation Forcing due to Atmospheric Aerosols

NASA Astrophysics Data System (ADS)

Sreenivas, K. R.; Singh, D. K.; Ponnulakshmi, V. K.; Subramanian, G.

2011-11-01

Micro-meteorological processes in the nocturnal atmospheric boundary layer (NBL) including the formation of radiation-fog and the development of inversion layers are controlled by heat transfer and the vertical temperature distribution close to the ground. In a recent study, it has been shown that the temperature profile close to the ground in stably-stratified, NBL is controlled by the radiative forcing due to suspended aerosols. Estimating aerosol forcing is also important in geo-engineering applications to evaluate the use of aerosols to mitigate greenhouse effects. Modeling capability in the above scenarios is limited by our knowledge of this forcing. Here, the design of an experimental setup is presented which can be used for evaluating the IR-radiation forcing on aerosols under either Rayleigh-Benard condition or under conditions corresponding to the NBL. We present results indicating the effect of surface emissivities of the top and bottom boundaries and the aerosol concentration on the temperature profiles. In order to understand the observed enhancement of the convection-threshold, we have determined the conduction-radiation time constant of an aerosol laden air layer. Our results help to explain observed temperature profiles in the NBL, the apparent stability of such profiles and indicate the need to account for the effect of aerosols in climatic/weather models.

Exploring the Longwave Radiative Effects of Dust Aerosols

NASA Technical Reports Server (NTRS)

Hansell, Richard A., Jr.

2012-01-01

Dust aerosols not only affect air quality and visibility where they pose a significant health and safety risk, but they can also play a role in modulating the energy balance of the Earth-atmosphere system by directly interacting with local radiative fields. Consequently, dust aerosols can impact regional climate patterns such as changes in precipitation and the evolution of the hydrological cycle. Assessing the direct effect of dust aerosols at the solar wavelengths is fairly straightforward due in part to the relatively large signal-to-noise ratio in broadband irradiance measurements. The longwave (LW) impacts, on the other hand, are rather difficult to ascertain since the measured dust signal level (10 Wm-2) is on the same order as the instrumental uncertainties. Moreover, compared to the shortwave (SW), limited experimental data on the LW optical properties of dust makes it a difficult challenge for constraining the LW impacts. Owing to the strong absorption features found in many terrestrial minerals (e.g., silicates and clays), the LW effects, although much smaller in magnitude compared to the SW, can still have a sizeable impact on the energetics of the Earth-atmosphere system, which can potentially trigger changes in the heat and moisture surface budgets, and dynamics of the atmosphere. The current endeavor is an integral part of an on-going research study to perform detailed assessments of dust direct aerosol radiative effects (DARE) using comprehensive global datasets from NASA Goddards mobile ground-based facility (cf. http://smartlabs.gsfc.nasa.gov/) during previous field experiments near key dust source regions. Here we examine and compare the results from two of these studies: the 2006 NASA African Monsoon Multidisciplinary Activities and the 2008 Asian Monsoon Years. The former study focused on transported Saharan dust at Sal Island (16.73N, 22.93W), Cape Verde along the west coast of Africa while the latter focused on Asian dust at Zhangye China (39

The direct effect of aerosols on solar radiation over the broader Mediterranean basin

NASA Astrophysics Data System (ADS)

Papadimas, C. D.; Hatzianastassiou, N.; Matsoukas, C.; Kanakidou, M.; Mihalopoulos, N.; Vardavas, I.

2011-11-01

For the first time, the direct radiative effect (DRE) of aerosols on solar radiation is computed over the entire Mediterranean basin, one of the most climatically sensitive world regions, by using a deterministic spectral radiation transfer model (RTM). The DRE effects on the outgoing shortwave radiation at the top of atmosphere (TOA), DRETOA, on the absorption of solar radiation in the atmospheric column, DREatm, and on the downward and absorbed surface solar radiation (SSR), DREsurf and DREnetsurf, respectively, are computed separately. The model uses input data for the period 2000-2007 for various surface and atmospheric parameters, taken from satellite (International Satellite Cloud Climatology Project, ISCCP-D2), Global Reanalysis projects (National Centers for Environmental Prediction - National Center for Atmospheric Research, NCEP/NCAR), and other global databases. The spectral aerosol optical properties (aerosol optical depth, AOD, asymmetry parameter, gaer and single scattering albedo, ωaer), are taken from the MODerate resolution Imaging Spectroradiometer (MODIS) of NASA (National Aeronautics and Space Administration) and they are Supplemented by the Global Aerosol Data Set (GADS). The model SSR fluxes have been successfully validated against measurements from 80 surface stations of the Global Energy Balance Archive (GEBA) covering the period 2000-2007. A planetary cooling is found above the Mediterranean on an annual basis (regional mean DRETOA = -2.4 Wm-2). Though planetary cooling is found over most of the region, up to -7 Wm-2, large positive DRETOA values (up to +25 Wm-2) are found over North Africa, indicating a strong planetary warming, as well as over the Alps (+0.5 Wm-2). Aerosols are found to increase the absorption of solar radiation in the atmospheric column over the region (DREatm = +11.1 Wm-2) and to decrease SSR (DREsurf = -16.5 Wm-2 and DREnetsurf -13.5 Wm-2) inducing thus significant atmospheric warming and surface radiative cooling

Analysis of Atmospheric Aerosol Data Sets and Application of Radiative Transfer Models to Compute Aerosol Effects

NASA Technical Reports Server (NTRS)

Schmid, Beat; Bergstrom, Robert W.; Redemann, Jens

2002-01-01

This report is the final report for "Analysis of Atmospheric Aerosol Data Sets and Application of Radiative Transfer Models to Compute Aerosol Effects". It is a bibliographic compilation of 29 peer-reviewed publications (published, in press or submitted) produced under this Cooperative Agreement and 30 first-authored conference presentations. The tasks outlined in the various proposals are listed below with a brief comment as to the research performed. Copies of title/abstract pages of peer-reviewed publications are attached.

Volcanic Aerosol Radiative Properties

NASA Technical Reports Server (NTRS)

Lacis, Andrew

2015-01-01

Large sporadic volcanic eruptions inject large amounts of sulfur bearing gases into the stratosphere which then get photochemically converted to sulfuric acid aerosol droplets that exert a radiative cooling effect on the global climate system lasting for several years.

Factors Affecting Aerosol Radiative Forcing

NASA Astrophysics Data System (ADS)

Wang, Jingxu; Lin, Jintai; Ni, Ruijing

2016-04-01

Rapid industrial and economic growth has meant a large amount of aerosols in the atmosphere with strong radiative forcing (RF) upon the climate system. Over parts of the globe, the negative forcing of aerosols has overcompensated for the positive forcing of greenhouse gases. Aerosol RF is determined by emissions and various chemical-transport-radiative processes in the atmosphere, a multi-factor problem whose individual contributors have not been well quantified. In this study, we analyze the major factors affecting RF of secondary inorganic aerosols (SIOAs, including sulfate, nitrate and ammonium), primary organic aerosol (POA), and black carbon (BC). We analyze the RF of aerosols produced by 11 major regions across the globe, including but not limited to East Asia, Southeast Asia, South Asia, North America, and Western Europe. Factors analyzed include population size, per capita gross domestic production (GDP), emission intensity (i.e., emissions per unit GDP), chemical efficiency (i.e., mass per unit emissions) and radiative efficiency (i.e., RF per unit mass). We find that among the 11 regions, East Asia produces the largest emissions and aerosol RF, due to relatively high emission intensity and a tremendous population size. South Asia produce the second largest RF of SIOA and BC and the highest RF of POA, in part due to its highest chemical efficiency among all regions. Although Southeast Asia also has large emissions, its aerosol RF is alleviated by its lowest chemical efficiency. The chemical efficiency and radiative efficiency of BC produced by the Middle East-North Africa are the highest across the regions, whereas its RF is lowered by a small per capita GDP. Both North America and Western Europe have low emission intensity, compensating for the effects on RF of large population sizes and per capita GDP. There has been a momentum to transfer industries to Southeast Asia and South Asia, and such transition is expected to continue in the coming years. The

Factors Affecting Aerosol Radiative Forcing

NASA Astrophysics Data System (ADS)

Wang, J.; Lin, J.; Ni, R.

2016-12-01

Rapid industrial and economic growth has meant large amount of aerosols in the atmosphere with strong radiative forcing (RF) upon the climate system. Over parts of the globe, the negative forcing of aerosols has overcompensated for the positive forcing of greenhouse gases. Aerosol RF is determined by emissions and various chemical-transport-radiative processes in the atmosphere, a multi-factor problem whose individual contributors have not been well quantified. In this study, we analyze the major factors affecting RF of secondary inorganic aerosols (SIOAs, including sulfate, nitrate and ammonium), primary organic aerosol (POA), and black carbon (BC). We analyze the RFof aerosols produced by 11 major regions across the globe, including but not limited to East Asia, Southeast Asia, South Asia, North America, and Western Europe. Factors analyzed include population size, per capita gross domestic production (GDP), emission intensity (i.e., emissionsper unit GDP), chemical efficiency (i.e., mass per unit emissions) and radiative efficiency (i.e., RF per unit mass). We find that among the 11 regions, East Asia produces the largest emissions and aerosol RF, due to relatively high emission intensity and a tremendous population size.South Asia produce the second largest RF of SIOA and BC and the highest RF of POA, in part due to its highest chemical efficiency among all regions. Although Southeast Asia also has large emissions,its aerosol RF is alleviated by its lowest chemical efficiency.The chemical efficiency and radiative efficiency of BC produced by the Middle East-North Africa are the highest across the regions, whereas its RF is loweredbyasmall per capita GDP.Both North America and Western Europe have low emission intensity, compensating for the effects on RF of large population sizes and per capita GDP. There has been a momentum to transfer industries to Southeast Asia and South Asia, and such transition is expected to continue in the coming years. The resulting

Simulation of Aerosol Transport and Radiative Effects In Lmd-gcm During Indoex-ifp 1999

NASA Astrophysics Data System (ADS)

Reddy, M. S.; Boucher, O.; Léon, J.-F.; Venkataraman, C.; Pham, M.

During the January-March 1999, an international collaborative field experiment, In- dian Ocean Experiment (INDOEX) was carried out to understand the anthropogenic aerosol effects on radiative forcing (Ramanathan, 2001). In the present work we sim- ulated the cycle of the multi-component aerosol (sulphate, black carbon, organic car- bon, dust, sea-salt and fly-ash) in the Laboratoire de Météorologie Dynamique General Circulation Model (LMD GCM) and estimated the consequent radiative forcing. Sim- ulations are carried out in the zoomed version of the model focusing on the Indian sub- continent and Indian Ocean regions, for January-April 1999. To account correctly for the aerosol emissions in the source regions (Indian subcontinent) we have integrated newly developed SO2 and aerosol emission inventory for India for 1999 (Reddy and Venkataraman, 2002a and b) into the global emission data set input to model. Model performance is evaluated by comparing the simulated aerosol concentration fields against measurements over continental and oceanic stations. Model predicted concentrations agree well in the oceanic stations but are in the lower end of mea- surements in the continental stations. A large plume of sulphate and other aerosols ex- tended from the Indian sub-continent into the Indian Ocean, from surface and elevated flows, extending down to 5S in the pristine southern Indian Ocean. Predicted spec- trally resolved aerosol optical depths (AOD) will be compared with sun-photometer measurements in the region. We also present a comparison of model predicted aerosol optical depths with satellite (Meteosat) derived AOD for the same period. An assess- ment of the multi-component aerosol radiative forcing will be made and results will be discussed in the context of the possible climate effects over the region. Finally, the regional source contributions to sulphate and carbonaceous aerosol loadings in the Indian Ocean will be presented.

Use of A-Train Aerosol Observations to Constrain Direct Aerosol Radiative Effects (DARE) Comparisons with Aerocom Models and Uncertainty Assessments

NASA Technical Reports Server (NTRS)

Redemann, J.; Shinozuka, Y.; Kacenelenbogen, M.; Segal-Rozenhaimer, M.; LeBlanc, S.; Vaughan, M.; Stier, P.; Schutgens, N.

2017-01-01

We describe a technique for combining multiple A-Train aerosol data sets, namely MODIS spectral AOD (aerosol optical depth), OMI AAOD (absorption aerosol optical depth) and CALIOP aerosol backscatter retrievals (hereafter referred to as MOC retrievals) to estimate full spectral sets of aerosol radiative properties, and ultimately to calculate the 3-D distribution of direct aerosol radiative effects (DARE). We present MOC results using almost two years of data collected in 2007 and 2008, and show comparisons of the aerosol radiative property estimates to collocated AERONET retrievals. Use of the MODIS Collection 6 AOD data derived with the dark target and deep blue algorithms has extended the coverage of the MOC retrievals towards higher latitudes. The MOC aerosol retrievals agree better with AERONET in terms of the single scattering albedo (ssa) at 441 nm than ssa calculated from OMI and MODIS data alone, indicating that CALIOP aerosol backscatter data contains information on aerosol absorption. We compare the spatio-temporal distribution of the MOC retrievals and MOC-based calculations of seasonal clear-sky DARE to values derived from four models that participated in the Phase II AeroCom model intercomparison initiative. Overall, the MOC-based calculations of clear-sky DARE at TOA over land are smaller (less negative) than previous model or observational estimates due to the inclusion of more absorbing aerosol retrievals over brighter surfaces, not previously available for observationally-based estimates of DARE. MOC-based DARE estimates at the surface over land and total (land and ocean) DARE estimates at TOA are in between previous model and observational results. Comparisons of seasonal aerosol property to AeroCom Phase II results show generally good agreement best agreement with forcing results at TOA is found with GMI-MerraV3. We discuss sampling issues that affect the comparisons and the major challenges in extending our clear-sky DARE results to all

Effect of Aerosols on Surface Radiation and Air Quality in the Central American Region Estimated Using Satellite UV Instruments

NASA Astrophysics Data System (ADS)

Bhartia, P. K.; Torres, O.; Krotkov, N. A.

2007-05-01

Solar radiation reaching the Earth's surface is reduced by both aerosol scattering and aerosol absorption. Over many parts of the world the latter effect can be as large or larger than the former effect, and small changes in the aerosol single scattering albedo can either cancel the former effect or enhance it. In addition, absorbing aerosols embedded in clouds can greatly reduce the amount of radiation reaching the surface by multiple scattering. Though the potential climatic effects of absorbing aerosols have received considerable attention lately, their effect on surface UV, photosynthesis, and photochemistry can be equally important for our environment and may affect human health and agricultural productivity. Absorption of all aerosols commonly found in the Earth's atmosphere becomes larger in the UV and blue wavelengths and has a relatively strong wavelength dependence. This is particularly true of mineral dust and organic aerosols. However, these effects have been very difficult to estimate on a global basis since the satellite instruments that operate in the visible are primarily sensitive to aerosol scattering. A notable exception is the UV Aerosol Index (AI), first produced using NASA's Nimbus-7 TOMS data. AI provides a direct measure of the effect of aerosol absorption on the backscattered UV radiation in both clear and cloudy conditions, as well as over snow/ice. Although many types of aerosols produce a distinct color cast in the visible images, and aerosols absorption over clouds and snow/ice could, in principle be detected from their color, so far this technique has worked well only in the UV. In this talk we will discuss what we have learned from the long-term record of AI produced from TOMS and Aura/OMI about the possible role of aerosols on surface radiation and air quality in the Central American region.

Aerosol Radiative Forcing Derived From SeaWIFS - Retrieved Aerosol Optical Properties

NASA Technical Reports Server (NTRS)

Chou, Mong-Dah; Chan, Pui-King; Wang, Menghua; Einaudi, Franco (Technical Monitor)

2000-01-01

To understand climatic implications of aerosols over global oceans, the aerosol optical properties retrieved from the Sea-viewing Wide Field-of-view Sensor (SeaWiFS) are analyzed, and the effects of the aerosols on the Earth's radiation budgets (aerosol radiative forcing, ARF) are computed using a radiative transfer model. It is found that the distribution of the SeaWiFS-retrieved aerosol optical thickness is distinctively zonal. The maximum in the equatorial region coincides with the Intertropical Convergence Zone, and the maximum in the Southern Hemispheric high latitudes coincides with the region of prevailing westerlies. The minimum aerosol optical thickness is found in the subtropical high pressure regions, especially in the Southern Hemisphere. These zonal patterns clearly demonstrate the influence of atmospheric circulation on the oceanic aerosol distribution. Over global oceans, aerosols reduce the annual mean net downward solar flux by 5.4 W m-2 at the top of the atmosphere and by 6.1 W m-2 at the surface. The largest ARF is found in the tropical Atlantic, Arabian Sea, Bay of Bengal, the coastal regions of Southeast and East Asia, and the Southern Hemispheric high latitudes. During the period of the Indonesian big fires (September-December 1997), the cooling due to aerosols is greater than 15 W m-2 at the top of the atmosphere and greater than 30 W m(exp -1) at the surface in the vicinity of the maritime continents. The atmosphere receives extra solar radiation by greater than 15 W m(exp -1) over a large area. These large changes in radiative fluxes are expected to have enhanced the atmospheric stability, weakened the atmospheric circulation, and augmented the drought condition during that period. It would be very instructive to simulate the regional climatic. The model-calculated clear sky solar flux at the top of the atmosphere is compared with that derived from the Clouds and the Earth's Radiant Energy System (CERES). The net downward solar flux of

Influence of Observed Diurnal Cycles of Aerosol Optical Depth on Aerosol Direct Radiative Effect

NASA Technical Reports Server (NTRS)

Arola, A.; Eck, T. F.; Huttunen, J.; Lehtinen, K. E. J.; Lindfors, A. V.; Myhre, G.; Smirinov, A.; Tripathi, S. N.; Yu, H.

2013-01-01

The diurnal variability of aerosol optical depth (AOD) can be significant, depending on location and dominant aerosol type. However, these diurnal cycles have rarely been taken into account in measurement-based estimates of aerosol direct radiative forcing (ADRF) or aerosol direct radiative effect (ADRE). The objective of our study was to estimate the influence of diurnal aerosol variability at the top of the atmosphere ADRE estimates. By including all the possible AERONET sites, we wanted to assess the influence on global ADRE estimates. While focusing also in more detail on some selected sites of strongest impact, our goal was to also see the possible impact regionally.We calculated ADRE with different assumptions about the daily AOD variability: taking the observed daily AOD cycle into account and assuming diurnally constant AOD. Moreover, we estimated the corresponding differences in ADREs, if the single AOD value for the daily mean was taken from the the Moderate Resolution Imaging Spectroradiometer (MODIS) Terra or Aqua overpass times, instead of accounting for the true observed daily variability. The mean impact of diurnal AOD variability on 24 h ADRE estimates, averaged over all AERONET sites, was rather small and it was relatively small even for the cases when AOD was chosen to correspond to the Terra or Aqua overpass time. This was true on average over all AERONET sites, while clearly there can be much stronger impact in individual sites. Examples of some selected sites demonstrated that the strongest observed AOD variability (the strongest morning afternoon contrast) does not typically result in a significant impact on 24 h ADRE. In those cases, the morning and afternoon AOD patterns are opposite and thus the impact on 24 h ADRE, when integrated over all solar zenith angles, is reduced. The most significant effect on daily ADRE was induced by AOD cycles with either maximum or minimum AOD close to local noon. In these cases, the impact on 24 h ADRE was

On Effective Radiative Forcing of Partial Internally and Externally Mixed Aerosols and Their Effects on Global Climate

NASA Astrophysics Data System (ADS)

Zhou, Chen; Zhang, Hua; Zhao, Shuyun; Li, Jiangnan

2018-01-01

The total effective radiative forcing (ERF) due to partial internally mixed (PIM) and externally mixed (EM) anthropogenic aerosols, as well as their climatic effects since the year of 1850, was evaluated and compared using the aerosol-climate online coupled model of BCC_AGCM2.0_CUACE/Aero. The influences of internal mixing (IM) on aerosol hygroscopicity parameter, optical properties, and concentration were considered. Generally, IM could markedly weaken the negative ERF and cooling effects of anthropogenic aerosols. The global annual mean ERF of EM anthropogenic aerosols from 1850 to 2010 was -1.87 W m-2, of which the aerosol-radiation interactive ERF (ERFari) and aerosol-cloud interactive ERF (ERFaci) were -0.49 and -1.38 W m-2, respectively. The global annual mean ERF due to PIM anthropogenic aerosols from 1850 to 2010 was -1.23 W m-2, with ERFari and ERFaci of -0.23 and -1.01 W m-2, respectively. The global annual mean surface temperature and water evaporation and precipitation were reduced by 1.74 K and 0.14 mm d-1 for EM scheme and 1.28 K and 0.11 mm d-1 for PIM scheme, respectively. However, the relative humidity near the surface was slightly increased for both mixing cases. The Intertropical Convergence Zone was southwardly shifted for both EM and PIM cases but was less southwardly shifted in PIM scheme due to the less reduction in atmospheric temperature in the midlatitude and low latitude of the Northern Hemisphere.

Host Model Uncertainty in Aerosol Radiative Forcing Estimates - The AeroCom Prescribed Experiment

NASA Astrophysics Data System (ADS)

Stier, P.; Kinne, S.; Bellouin, N.; Myhre, G.; Takemura, T.; Yu, H.; Randles, C.; Chung, C. E.

2012-04-01

Anthropogenic and natural aerosol radiative effects are recognized to affect global and regional climate. However, even for the case of identical aerosol emissions, the simulated direct aerosol radiative forcings show significant diversity among the AeroCom models (Schulz et al., 2006). Our analysis of aerosol absorption in the AeroCom models indicates a larger diversity in the translation from given aerosol radiative properties (absorption optical depth) to actual atmospheric absorption than in the translation of a given atmospheric burden of black carbon to the radiative properties (absorption optical depth). The large diversity is caused by differences in the simulated cloud fields, radiative transfer, the relative vertical distribution of aerosols and clouds, and the effective surface albedo. This indicates that differences in host model (GCM or CTM hosting the aerosol module) parameterizations contribute significantly to the simulated diversity of aerosol radiative forcing. The magnitude of these host model effects in global aerosol model and satellites retrieved aerosol radiative forcing estimates cannot be estimated from the diagnostics of the "standard" AeroCom forcing experiments. To quantify the contribution of differences in the host models to the simulated aerosol radiative forcing and absorption we conduct the AeroCom Prescribed experiment, a simple aerosol model and satellite retrieval intercomparison with prescribed highly idealised aerosol fields. Quality checks, such as diagnostic output of the 3D aerosol fields as implemented in each model, ensure the comparability of the aerosol implementation in the participating models. The simulated forcing variability among the models and retrievals is a direct measure of the contribution of host model assumptions to the uncertainty in the assessment of the aerosol radiative effects. We will present the results from the AeroCom prescribed experiment with focus on the attribution to the simulated variability

Dust radiative effect over Europe, Mediterranean, Sahara and Middle East from a radiative transfer model using BSC-DREAM8b aerosol optical data

NASA Astrophysics Data System (ADS)

Papadimas, Christos; Gkikas, Antonis; Hatzianastassiou, Nikos; Matsoukas, Christos; Kazadzis, Stelios; Basart, Sara; Baldasano, Jose; Vardavas, Ilias

2013-04-01

The arid regions of Saharan desert and Middle East are the world's major dust sources. However, dust particles from these areas are transported to nearby regions, through favourable synoptic conditions, even reaching remote locations in Europe or in the Arctic. This transport is very important in numerous aspects. One of its most important effects is on the radiation budget, and more specifically on solar radiation, through the aerosol direct radiative effect (DRE). Previous studies have shown that this effect is great under dust load conditions. Therefore, it is very important to simulate dust transport processes and associated radiative effects. The simulation of dust production, transport and removal is done by numerical models, which however have their own limitations as to the consideration of physical and dynamical processes as well as their initial conditions. On the other hand, the computation of dust DRE is ideally done with radiative transfer models (RTMs), which however imply uncertainties associated with the input aerosol optical properties. The most important aerosol optical properties used in RTMs and climate models are aerosol optical depth (AOD), single scattering albedo (SSA) and asymmetry parameter (AP). The main target of the present study is to reduce the uncertainties of dust DRE by using a detailed spectral RTM and an acknowledged regional and meso-scale model describing the distribution of dust. The combined use of these tools is applied to the region covering the deserts of Sahara, Arabian Peninsula and Middle East, and the neighbouring Mediterranean basin and European continent (extending from 15°N to 60°N and from 21°W to 54°E). The computations are performed on a monthly mean basis, refer to the 11-year period 2000-2010, and quantify the effects of dust on the reflected solar radiation at the top of atmosphere (DRETOA), on the absorbed solar radiation within the atmosphere (DREatmab), and on the downwelling and absorbed solar

Multi-Decadal Change of Atmospheric Aerosols and Their Effect on Surface Radiation

NASA Technical Reports Server (NTRS)

Chin, Mian; Diehl, Thomas; Tan, Qian; Wild, Martin; Qian, Yun; Yu, Hongbin; Bian, Huisheng; Wang, Weiguo

2012-01-01

We present an investigation on multi-decadal changes of atmospheric aerosols and their effects on surface radiation using a global chemistry transport model along with the near-term to long-term data records. We focus on a 28-year time period of satellite era from 1980 to 2007, during which a suite of aerosol data from satellite observations and ground-based remote sensing and in-situ measurements have become available. We analyze the long-term global and regional aerosol optical depth and concentration trends and their relationship to the changes of emissions" and assess the role aerosols play in the multi-decadal change of solar radiation reaching the surface (known as "dimming" or "brightening") at different regions of the world, including the major anthropogenic source regions (North America, Europe, Asia) that have been experiencing considerable changes of emissions, dust and biomass burning regions that have large interannual variabilities, downwind regions that are directly affected by the changes in the source area, and remote regions that are considered to representing "background" conditions.

Investigation of Multi-decadal Trends in Aerosol Direct Radiative Effects over North America using a Coupled Meteorology-Chemistry Model

NASA Astrophysics Data System (ADS)

Mathur, R.; Pleim, J.; Wong, D.; Wei, C.; Xing, J.; Gan, M.; Yu, S.; Binkowski, F.

2012-12-01

While aerosol radiative effects have been recognized as some of the largest sources of uncertainty among the forcers of climate change, there has been little effort devoted to verification of the spatial and temporal variability of the magnitude and directionality of aerosol radiative forcing. A comprehensive investigation of the processes regulating aerosol distributions, their optical properties, and their radiative effects and verification of their simulated effects for past conditions relative to measurements is needed in order to build confidence in the estimates of the projected impacts arising from changes in both anthropogenic forcing and climate change. This study aims at addressing this issue through a systematic investigation of changes in anthropogenic emissions of SO2 and NOx over the past two decades in the United States, their impacts on anthropogenic aerosol loading in the North American troposphere, and subsequent impacts on regional radiation budgets. A newly developed 2-way coupled meteorology and air pollution model composed of the Weather Research and Forecasting (WRF) model and the Community Multiscale Air Quality (CMAQ) model is being run for 20 years (1990 - 2010) on a 12 km resolution grid that covers most of North America including the entire conterminous US. During this period US emissions of SO2 and NOx have been reduced by about 66% and 50%, respectively, mainly due to Title IV of the U.S. Clean Air Act Amendments (CAA) that aimed to reduce emissions that contribute to acid deposition. A methodology is developed to consistently estimate emission inventories for the 20-year period accounting for air quality regulations as well as population trends, economic conditions, and technology changes in motor vehicles and electric power generation. The coupled WRF-CMAQ model includes detailed treatment of direct effects of aerosols on photolysis rates as well as on shortwave radiation and the direct effects of tropospheric ozone on the long

Estimation of Aerosol Direct Radiative Effects Over the Mid-Latitude North Atlantic from Satellite and In Situ Measurements

NASA Technical Reports Server (NTRS)

Bergstrom, Robert W.; Russell, P. B.

2000-01-01

We estimate solar radiative flux changes due to aerosols over the mid-latitude North Atlantic by combining optical depths from AVHRR measurements with aerosol properties from the recent TARFOX program. Results show that, over the ocean the aerosol decreases the net radiative flux at the tropopause and therefore has a cooling effect. Cloud-free, 24-hour average flux changes range from -9 W/sq m near the eastern US coast in summer to -1 W/sq m in the mid-Atlantic during winter. Cloud-free North Atlantic regional averages range from -5.1 W/sq m in summer to -1.7 W/sq m in winter, with an annual average of -3.5 W/sq m. Cloud effects estimated from ISCCP data, reduce the regional annual average to -0.8 W/sq m. All values are for the moderately absorbing TARFOX aerosol (omega(0.55 microns) = 0.9); values for a nonabsorbing aerosol are approx. 30% more negative. We compare our results to a variety of other calculations of aerosol radiative effects.

Potential sensitivity of photosynthesis and isoprene emission to direct radiative effects of atmospheric aerosol pollution

NASA Astrophysics Data System (ADS)

Strada, Susanna; Unger, Nadine

2016-04-01

A global Earth system model is applied to quantify the impacts of direct anthropogenic aerosol effective radiative forcing on gross primary productivity (GPP) and isoprene emission. The impacts of different pollution aerosol sources (anthropogenic, biomass burning, and non-biomass burning) are investigated by performing sensitivity experiments. The model framework includes all known light and meteorological responses of photosynthesis, but uses fixed canopy structures and phenology. On a global scale, our results show that global land carbon fluxes (GPP and isoprene emission) are not sensitive to pollution aerosols, even under a global decline in surface solar radiation (direct + diffuse) by ˜ 9 %. At a regional scale, GPP and isoprene emission show a robust but opposite sensitivity to pollution aerosols in regions where forested canopies dominate. In eastern North America and Eurasia, anthropogenic pollution aerosols (mainly from non-biomass burning sources) enhance GPP by +5-8 % on an annual average. In the northwestern Amazon Basin and central Africa, biomass burning aerosols increase GPP by +2-5 % on an annual average, with a peak in the northwestern Amazon Basin during the dry-fire season (+5-8 %). The prevailing mechanism varies across regions: light scattering dominates in eastern North America, while a reduction in direct radiation dominates in Europe and China. Aerosol-induced GPP productivity increases in the Amazon and central Africa include an additional positive feedback from reduced canopy temperatures in response to increases in canopy conductance. In Eurasia and northeastern China, anthropogenic pollution aerosols drive a decrease in isoprene emission of -2 to -12 % on an annual average. Future research needs to incorporate the indirect effects of aerosols and possible feedbacks from dynamic carbon allocation and phenology.

Does temperature nudging overwhelm aerosol radiative effects in regional integrated climate models?

NASA Astrophysics Data System (ADS)

He, Jian; Glotfelty, Timothy; Yahya, Khairunnisa; Alapaty, Kiran; Yu, Shaocai

2017-04-01

Nudging (data assimilation) is used in many regional integrated meteorology-air quality models to reduce biases in simulated climatology. However, in such modeling systems, temperature changes due to nudging could compete with temperature changes induced by radiatively active and hygroscopic short-lived tracers leading to two interesting dilemmas: when nudging is continuously applied, what are the relative sizes of these two radiative forces at regional and local scales? How do these two forces present in the free atmosphere differ from those present at the surface? This work studies these two issues by converting temperature changes due to nudging into pseudo radiative effects (PRE) at the surface (PRE_sfc), in troposphere (PRE_atm), and at the top of atmosphere (PRE_toa), and comparing PRE with the reported aerosol radiative effects (ARE). Results show that the domain-averaged PRE_sfc is smaller than ARE_sfc estimated in previous studies and this work, but could be significantly larger than ARE_sfc at local scales. PRE_atm is also much smaller than ARE_atm. These results indicate that appropriate nudging methodology could be applied to the integrated models to study aerosol radiative effects at continental/regional scales, but it should be treated with caution for local scale applications.

“Modeling Trends in Aerosol Direct Radiative Effects over the Northern Hemisphere using a Coupled Meteorology-Chemistry Model”

EPA Science Inventory

While aerosol radiative effects have been recognized as some of the largest sources of uncertainty among the forcers of climate change, the verification of the spatial and temporal variability of the magnitude and directionality of aerosol radiative forcing has remained challengi...

New approaches to quantifying aerosol influence on the cloud radiative effect

PubMed Central

Feingold, Graham; McComiskey, Allison; Yamaguchi, Takanobu; Johnson, Jill S.; Carslaw, Kenneth S.; Schmidt, K. Sebastian

2016-01-01

The topic of cloud radiative forcing associated with the atmospheric aerosol has been the focus of intense scrutiny for decades. The enormity of the problem is reflected in the need to understand aspects such as aerosol composition, optical properties, cloud condensation, and ice nucleation potential, along with the global distribution of these properties, controlled by emissions, transport, transformation, and sinks. Equally daunting is that clouds themselves are complex, turbulent, microphysical entities and, by their very nature, ephemeral and hard to predict. Atmospheric general circulation models represent aerosol−cloud interactions at ever-increasing levels of detail, but these models lack the resolution to represent clouds and aerosol−cloud interactions adequately. There is a dearth of observational constraints on aerosol−cloud interactions. We develop a conceptual approach to systematically constrain the aerosol−cloud radiative effect in shallow clouds through a combination of routine process modeling and satellite and surface-based shortwave radiation measurements. We heed the call to merge Darwinian and Newtonian strategies by balancing microphysical detail with scaling and emergent properties of the aerosol−cloud radiation system. PMID:26831092

An Investigation of the Radiative Effects and Climate Feedbacks of Sea Ice Sources of Sea Salt Aerosol

NASA Astrophysics Data System (ADS)

Horowitz, H. M.; Alexander, B.; Bitz, C. M.; Jaegle, L.; Burrows, S. M.

2017-12-01

In polar regions, sea ice is a major source of sea salt aerosol through lofting of saline frost flowers or blowing saline snow from the sea ice surface. Under continued climate warming, an ice-free Arctic in summer with only first-year, more saline sea ice in winter is likely. Previous work has focused on climate impacts in summer from increasing open ocean sea salt aerosol emissions following complete sea ice loss in the Arctic, with conflicting results suggesting no net radiative effect or a negative climate feedback resulting from a strong first aerosol indirect effect. However, the radiative forcing from changes to the sea ice sources of sea salt aerosol in a future, warmer climate has not previously been explored. Understanding how sea ice loss affects the Arctic climate system requires investigating both open-ocean and sea ice sources of sea-salt aerosol and their potential interactions. Here, we implement a blowing snow source of sea salt aerosol into the Community Earth System Model (CESM) dynamically coupled to the latest version of the Los Alamos sea ice model (CICE5). Snow salinity is a key parameter affecting blowing snow sea salt emissions and previous work has assumed constant regional snow salinity over sea ice. We develop a parameterization for dynamic snow salinity in the sea ice model and examine how its spatial and temporal variability impacts the production of sea salt from blowing snow. We evaluate and constrain the snow salinity parameterization using available observations. Present-day coupled CESM-CICE5 simulations of sea salt aerosol concentrations including sea ice sources are evaluated against in situ and satellite (CALIOP) observations in polar regions. We then quantify the present-day radiative forcing from the addition of blowing snow sea salt aerosol with respect to aerosol-radiation and aerosol-cloud interactions. The relative contributions of sea ice vs. open ocean sources of sea salt aerosol to radiative forcing in polar regions is

Aerosol radiative effects on mesoscale cloud-precipitation variables over Northeast Asia during the MAPS-Seoul 2015 campaign

NASA Astrophysics Data System (ADS)

Park, Shin-Young; Lee, Hyo-Jung; Kang, Jeong-Eon; Lee, Taehyoung; Kim, Cheol-Hee

2018-01-01

The online model, Weather Research and Forecasting Model with Chemistry (WRF-Chem) is employed to interpret the effects of aerosol-cloud-precipitation interaction on mesoscale meteorological fields over Northeast Asia during the Megacity Air Pollution Study-Seoul (MAPS-Seoul) 2015 campaign. The MAPS-Seoul campaign is a pre-campaign of the Korea-United States Air Quality (KORUS-AQ) campaign conducted over the Korean Peninsula. We validated the WRF-Chem simulations during the campaign period, and analyzed aerosol-warm cloud interactions by diagnosing both aerosol direct, indirect, and total effects. The results demonstrated that aerosol directly decreased downward shortwave radiation up to -44% (-282 W m-2) for this period and subsequently increased downward longwave radiation up to +15% (∼52 W m-2) in the presence of low-level clouds along the thematic area. Aerosol increased cloud fraction indirectly up to ∼24% with the increases of both liquid water path and the droplet number mixing ratio. Precipitation properties were altered both directly and indirectly. Direct effects simply changed cloud-precipitation quantities via simple updraft process associated with perturbed radiation and temperature, while indirect effects mainly suppressed precipitation, but sometimes increased precipitation in the higher relative humidity atmosphere or near vapor-saturated condition. The total aerosol effects caused a time lag of the precipitation rate with the delayed onset time of up to 9 h. This implies the importance of aerosol effects in improving mesoscale precipitation rate prediction in the online approach in the presence of non-linear warm cloud.

Estimation of Asian Dust Aerosol Effect on Cloud Radiation Forcing Using Fu-Liou Radiative Model and CERES Measurements

NASA Technical Reports Server (NTRS)

Su, Jing; Huang, Jianping; Fu, Qiang; Minnis, Patrick; Ge, Jinming; Bi, Jianrong

2008-01-01

The impact of Asian dust on cloud radiative forcing during 2003-2006 is studied by using the Earth's Radiant Energy Budget Scanner (CERES) data and the Fu-Liou radiative transfer model. Analysis of satellite data shows that the dust aerosol significantly reduced the cloud cooling effect at TOA. In dust contaminated cloudy regions, the 4-year mean values of the instantaneous shortwave, longwave and net cloud radiative forcing are -138.9, 69.1, and -69.7 Wm(sup -2), which are 57.0, 74.2, and 46.3%, respectively, of the corresponding values in more pristine cloudy regions. The satellite-retrieved cloud properties are significantly different in the dusty regions and can influence the radiative forcing indirectly. The contributions to the cloud radiation forcing by the dust direct, indirect and semi-direct effects are estimated using combined satellite observations and Fu-Liou model simulation. The 4-year mean value of combination of indirect and semi-direct shortwave radiative forcing (SWRF) is 82.2 Wm(sup -2), which is 78.4% of the total dust effect. The direct effect is only 22.7 Wm(sup -2), which is 21.6% of the total effect. Because both first and second indirect effects enhance cloud cooling, the aerosol-induced cloud warming is mainly the result of the semi-direct effect of dust.

Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES)

NASA Astrophysics Data System (ADS)

Zaveri, R. A.; Shaw, W. J.; Cziczo, D. J.; Schmid, B.; Ferrare, R. A.; Alexander, M. L.; Alexandrov, M.; Alvarez, R. J.; Arnott, W. P.; Atkinson, D. B.; Baidar, S.; Banta, R. M.; Barnard, J. C.; Beranek, J.; Berg, L. K.; Brechtel, F.; Brewer, W. A.; Cahill, J. F.; Cairns, B.; Cappa, C. D.; Chand, D.; China, S.; Comstock, J. M.; Dubey, M. K.; Easter, R. C.; Erickson, M. H.; Fast, J. D.; Floerchinger, C.; Flowers, B. A.; Fortner, E.; Gaffney, J. S.; Gilles, M. K.; Gorkowski, K.; Gustafson, W. I.; Gyawali, M.; Hair, J.; Hardesty, R. M.; Harworth, J. W.; Herndon, S.; Hiranuma, N.; Hostetler, C.; Hubbe, J. M.; Jayne, J. T.; Jeong, H.; Jobson, B. T.; Kassianov, E. I.; Kleinman, L. I.; Kluzek, C.; Knighton, B.; Kolesar, K. R.; Kuang, C.; Kubátová, A.; Langford, A. O.; Laskin, A.; Laulainen, N.; Marchbanks, R. D.; Mazzoleni, C.; Mei, F.; Moffet, R. C.; Nelson, D.; Obland, M. D.; Oetjen, H.; Onasch, T. B.; Ortega, I.; Ottaviani, M.; Pekour, M.; Prather, K. A.; Radney, J. G.; Rogers, R. R.; Sandberg, S. P.; Sedlacek, A.; Senff, C. J.; Senum, G.; Setyan, A.; Shilling, J. E.; Shrivastava, M.; Song, C.; Springston, S. R.; Subramanian, R.; Suski, K.; Tomlinson, J.; Volkamer, R.; Wallace, H. W.; Wang, J.; Weickmann, A. M.; Worsnop, D. R.; Yu, X.-Y.; Zelenyuk, A.; Zhang, Q.

2012-08-01

Substantial uncertainties still exist in the scientific understanding of the possible interactions between urban and natural (biogenic) emissions in the production and transformation of atmospheric aerosol and the resulting impact on climate change. The US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program's Carbonaceous Aerosol and Radiative Effects Study (CARES) carried out in June 2010 in Central Valley, California, was a comprehensive effort designed to improve this understanding. The primary objective of the field study was to investigate the evolution of secondary organic and black carbon aerosols and their climate-related properties in the Sacramento urban plume as it was routinely transported into the forested Sierra Nevada foothills area. Urban aerosols and trace gases experienced significant physical and chemical transformations as they mixed with the reactive biogenic hydrocarbons emitted from the forest. Two heavily-instrumented ground sites - one within the Sacramento urban area and another about 40 km to the northeast in the foothills area - were set up to characterize the evolution of meteorological variables, trace gases, aerosol precursors, aerosol size, composition, and climate-related properties in freshly polluted and "aged" urban air. On selected days, the DOE G-1 aircraft was deployed to make similar measurements upwind and across the evolving Sacramento plume in the morning and again in the afternoon. The NASA B-200 aircraft, carrying remote sensing instruments, was also deployed to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties within and around the plume. This overview provides: (a) the scientific background and motivation for the study, (b) the operational and logistical information pertinent to the execution of the study, (c) an overview of key observations and initial findings from the aircraft and ground-based sampling platforms, and (d) a roadmap of planned data

Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES)

NASA Astrophysics Data System (ADS)

Zaveri, R. A.; Shaw, W. J.; Cziczo, D. J.; Schmid, B.; Alexander, M. L.; Alexandrov, M.; Alvarez, R. J.; Arnott, W. P.; Atkinson, D. B.; Baidar, S.; Banta, R. M.; Barnard, J. C.; Beranek, J.; Berg, L. K.; Brechtel, F.; Brewer, W. A.; Cahill, J. F.; Cairns, B.; Cappa, C. D.; Chand, D.; China, S.; Comstock, J. M.; Dubey, M. K.; Easter, R. C.; Fast, J. D.; Floerchinger, C.; Flowers, B. A.; Fortner, E.; Gaffney, J. S.; Gilles, M. K.; Gorkowski, K.; Gustafson, W. I.; Gyawali, M.; Hair, J.; Hardesty, R. M.; Harworth, J. W.; Herndon, S.; Hiranuma, N.; Hostetler, C.; Hubbe, J. M.; Jayne, J. T.; Jeong, H.; Jobson, B. T.; Kleinman, L. I.; Kluzek, C.; Knighton, B.; Kolesar, K. R.; Kuang, C.; Langford, A. O.; Laskin, A.; Marchbanks, R. D.; Mazzoleni, C.; Mei, F.; Moffet, R. C.; Nelson, D.; Obland, M. D.; Oetjen, H.; Onasch, T. B.; Ortega, I.; Ottaviani, M.; Pekour, M.; Prather, K. A.; Radney, J. G.; Rogers, R. R.; Sandberg, S. P.; Sedlacek, A.; Senff, C. J.; Senum, G.; Setyan, A.; Shilling, J. E.; Shrivastava, M.; Song, C.; Springston, S. R.; Subramanian, R.; Tomlinson, J.; Volkamer, R.; Wallace, H. W.; Wang, J.; Weickmann, A. M.; Yu, X.-Y.; Zelenyuk, A.; Zhang, Q.

2012-01-01

Substantial uncertainties still exist in the scientific understanding of the possible interactions between urban and natural (biogenic) emissions in the production and transformation of atmospheric aerosol and the resulting impact on climate change. The US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program's Carbonaceous Aerosol and Radiative Effects Study (CARES) carried out in June 2010 in Central Valley, California, was a comprehensive effort designed to improve this understanding. The primary objective of the field study was to investigate the evolution of secondary organic and black carbon aerosols and their climate-related properties in the Sacramento urban plume as it was routinely transported into the forested Sierra Nevada foothills area. Urban aerosols and trace gases experienced significant physical and chemical transformations as they mixed with the reactive biogenic hydrocarbons emitted from the forest. Two heavily-instrumented ground sites - one within the Sacramento urban area and another about 40 km to the northeast in the foothills area - were set up to characterize the evolution of meteorological variables, trace gases, aerosol precursors, aerosol size, composition, and climate-related properties in freshly polluted and "aged" urban air. On selected days, the DOE G-1 aircraft was deployed to make similar measurements upwind and across the evolving Sacramento plume in the morning and again in the afternoon. The NASA B-200 aircraft, carrying remote sensing instruments, was also deployed to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties within and around the plume. This overview provides: (a) the scientific background and motivation for the study, (b) the operational and logistical information pertinent to the execution of the study, (c) an overview of key observations and initial results from the aircraft and ground-based sampling platforms, and (d) a roadmap of planned data

Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES)

NASA Technical Reports Server (NTRS)

Zaveri, R. A.; Shaw, W. J.; Cahill, J. F.; Cairns, Brian; Cappa, C. D.; Ottaviani, Matteo; Cziczo, D. J.; Ferrare, Richard A.; Alexander, M. L.; Alexandrov, Mikhail Dmitrievic;

Effects of aerosol from biomass burning on the global radiation budget

NASA Technical Reports Server (NTRS)

Penner, Joyce E.; Dickinson, Robert E.; O'Neill, Christine A.

1992-01-01

An analysis is made of the likely contribution of smoke particles from biomass burning to the global radiation balance. These particles act to reflect solar radiation directly; they also can act as cloud condensation nuclei, increasing the reflectivity of clouds. Together these effects, although uncertain, may add up globally to a cooling effect as large as 2 watts per square meter, comparable to the estimated contribution to sulfate aerosols. Anthropogenic increases of smoke emission thus may have helped weaken the net greenhouse warming from anthropogenic trace gases.

Radiative Effect of Springtime Biomass-Burning Aerosols over Northern Indochina During 7-SEAS Baseline 2013 Campaign

NASA Technical Reports Server (NTRS)

Pani, Shantanu Kumar; Wang, Sheng-Hsiang; Lin, Neng-Huei; Lee, Chung-Te; Tsay, Si-Chee; Holben, Brent N.; Janjai, Serm; Hsiao, Ta-Chih; Chuang, Ming-Tung; Chantara, Somporn

2016-01-01

The direct aerosol radiative effects of biomass-burning (BB) aerosols over northern Indochina were estimated by using aerosol properties (physical, chemical, and optical) along with the vertical profile measurements from ground-based measurements with integration of an optical and a radiative transfer model during the Seven South East Asian Studies Biomass-Burning Aerosols Stratocumulus Environment: Lifecycles Interactions Experiment (7-SEASBASELInE) conducted in spring 2013. Cluster analysis of backward trajectories showed the air masses arriving at mountainous background site (Doi Ang Khang; 19.93degN, 99.05degE, 1536 m above mean sea level) in northern Indochina, mainly from near-source inland BB activities and being confined in the planetary boundary layer. The PM(sub10) and black carbon (BC)mass were 87 +/- 28 and 7 +/- 2 micrograms m(exp -3), respectively. The aerosol optical depth (AOD (sub 500) was found to be 0.26--1.13 (0.71 +/- 0.24). Finer (fine mode fraction is approximately or equal to 0.95, angstrom-exponent at 440-870 nm is approximately or equal to 1.77) and significantly absorbing aerosols(single scattering albedo is approximately or equal to 0.89, asymmetry-parameter is approximately or equal to 0.67, and absorption AOD 0.1 at 440 nm) dominated over this region. BB aerosols (water soluble and BC) were the main contributor to the aerosol radiative forcing (ARF), while others (water insoluble, sea salt and mineral dust) were negligible mainly due to their low extinction efficiency. BC contributed only 6 to the surface aerosol mass but its contribution to AOD was 12 (2 times higher). The overall mean ARF was 8.0 and -31.4 W m(exp -2) at top-of-atmosphere (TOA) and at the surface (SFC), respectively. Likely, ARF due to BC was +10.7 and -18.1 W m(exp -2) at TOA and SFC, respectively. BC imposed the heating rate of +1.4 K d(exp -1) within the atmosphere and highlighting its pivotal role in modifying the radiation budget. We propose that to upgrade our

Radiative forcing and rapid adjustment of absorbing aerosols in the Pearl River Delta Region of China

NASA Astrophysics Data System (ADS)

Liu, Z.; Yim, S. H. L.; Lau, G.

2016-12-01

Part of organic carbon defined as brown carbon (BrC) has been found to absorb solar radiation, especially in near-ultraviolet and blue bands, but their radiation impact is far less understood than black carbon (BC). Rapid adjustment thought to occur within a few weeks, induced by aerosol radiative effect and thereby alter cloud cover or other climate components. These effects are particularly pronounced for absorbing aerosols. The data gathered is from an online coupled model, WRF-Chem. A two-simulation test is conducted from July 8 to July 15. The baseline simulation doesn't account for aerosol-radiation interactions, whereas the sensitivity run includes it. The differences between these two simulations represent total effects of the aerosol instantaneous radiative forcing and subsequent rapid adjustment. In Figure 1, without cloud effect (clear sky), at the top of atmosphere (TOA), the SW radiation changes are negative in the PRD region, representing an overall cooling effect of aerosols. However, in the atmosphere (ATM), aerosols heat the atmosphere by absorbing incoming solar radiation with an average of 2.4 W/m2 (Table 1). After including rapid adjustment (all sky), the radiation change pattern becomes significantly different, especially at TOA and surface (SFC). This may be caused by cloud cover change due to rapid adjustment. The magnitude of SW radiation changes for all sky at all levels is smaller than that for clear sky. This result suggests the rapid adjustment counteracts the instantaneous radiative forcing of aerosols. At TOA, the cooling effect of the aerosol is 74% lower for all sky compared with clear sky, highlighting an overall warming effect of rapid adjustment in the PRD region. Aerosol-induced changes (W/m2) TOA ATM SFC Clear Sky -9.2 2.4 -11.6 All Sky -2.4 1.9 -4.3 Table 1. Aerosol-induced averaged changes in shortwave radiation due to aerosol-radiation interactions in the Pearl River Delta. The test shows the rapid adjustment of aerosols

Aerosol Indirect Effects on Cirrus Clouds in Global Aerosol-Climate Models

NASA Astrophysics Data System (ADS)

Liu, X.; Zhang, K.; Wang, Y.; Neubauer, D.; Lohmann, U.; Ferrachat, S.; Zhou, C.; Penner, J.; Barahona, D.; Shi, X.

2015-12-01

Cirrus clouds play an important role in regulating the Earth's radiative budget and water vapor distribution in the upper troposphere. Aerosols can act as solution droplets or ice nuclei that promote ice nucleation in cirrus clouds. Anthropogenic emissions from fossil fuel and biomass burning activities have substantially perturbed and enhanced concentrations of aerosol particles in the atmosphere. Global aerosol-climate models (GCMs) have now been used to quantify the radiative forcing and effects of aerosols on cirrus clouds (IPCC AR5). However, the estimate uncertainty is very large due to the different representation of ice cloud formation and evolution processes in GCMs. In addition, large discrepancies have been found between model simulations in terms of the spatial distribution of ice-nucleating aerosols, relative humidity, and temperature fluctuations, which contribute to different estimates of the aerosol indirect effect through cirrus clouds. In this presentation, four GCMs with the start-of-the art representations of cloud microphysics and aerosol-cloud interactions are used to estimate the aerosol indirect effects on cirrus clouds and to identify the causes of the discrepancies. The estimated global and annual mean anthropogenic aerosol indirect effect through cirrus clouds ranges from 0.1 W m-2 to 0.3 W m-2 in terms of the top-of-the-atmosphere (TOA) net radiation flux, and 0.5-0.6 W m-2 for the TOA longwave flux. Despite the good agreement on global mean, large discrepancies are found at the regional scale. The physics behind the aerosol indirect effect is dramatically different. Our analysis suggests that burden of ice-nucleating aerosols in the upper troposphere, ice nucleation frequency, and relative role of ice formation processes (i.e., homogeneous versus heterogeneous nucleation) play key roles in determining the characteristics of the simulated aerosol indirect effects. In addition to the indirect effect estimate, we also use field campaign

Modeling Aerosol Microphysical and Radiative Effects on Clouds and Implications for the Effects of Black and Brown Carbon on Clouds

NASA Astrophysics Data System (ADS)

Ten Hoeve, J. E.; Jacobson, M. Z.

2010-12-01

Satellite observational studies have found an increase in cloud fraction (CF) and cloud optical depth (COD) with increasing aerosol optical depth (AOD) followed by a decreasing CF/COD with increasing AOD at higher AODs over the Amazon Basin. The shape of this curve is similar to that of a boomerang, and thus the effect has been dubbed the "boomerang effect.” The increase in CF/COD with increasing AOD at low AODs is ascribed to the first and second indirect effects and is referred to as a microphysical effect of aerosols on clouds. The decrease in CF/COD at higher AODs is ascribed to enhanced warming of clouds due to absorbing aerosols, either as inclusions in drops or interstitially between drops. This is referred to as a radiative effect. To date, the interaction of the microphysical and radiative effects has not been simulated with a regional or global computer model. Here, we simulate the boomerang effect with the nested global-through-urban climate, air pollution, weather forecast model, GATOR-GCMOM, for the Amazon biomass burning season of 2006. We also compare the model with an extensive set of data, including satellite data from MODIS, TRMM, and CALIPSO, in situ surface observations, upper-air data, and AERONET data. Biomass burning emissions are obtained from the Global Fire Emissions Database (GFEDv2), and are combined with MODIS land cover data along with biomass burning emission factors. A high-resolution domain, nested within three increasingly coarser domains, is employed over the heaviest biomass burning region within the arc of deforestation. Modeled trends in cloud properties with aerosol loading compare well with MODIS observed trends, allowing causation of these observed correlations, including of the boomerang effect, to be determined by model results. The impact of aerosols on various cloud parameters, such as cloud optical thickness, cloud fraction, cloud liquid water/ice content, and precipitation, are shown through differences between

Effects of morphology on the radiative properties of internally mixed light absorbing carbon aerosols with different aging status.

PubMed

Cheng, Tianhai; Wu, Yu; Chen, Hao

2014-06-30

Light absorbing carbon aerosols play a substantial role in climate change through radiative forcing, which is the dominant absorber of solar radiation. Radiative properties of light absorbing carbon aerosols are strongly dependent on the morphological factors and the mixing mechanism of black carbon with other aerosol components. This study focuses on the morphological effects on the optical properties of internally mixed light absorbing carbon aerosols using the numerically exact superposition T-matrix method. Three types aerosols with different aging status such as freshly emitted BC particles, thinly coated light absorbing carbon aerosols, heavily coated light absorbing carbon aerosols are studied. Our study showed that morphological factors change with the aging of internally mixed light absorbing carbon aerosols to result in a dramatic change in their optical properties. The absorption properties of light absorbing carbon aerosols can be enhanced approximately a factor of 2 at 0.67 um, and these enhancements depend on the morphological factors. A larger shell/core diameter ratio of volume-equivalent shell-core spheres (S/C), which indicates the degree of coating, leads to stronger absorption. The enhancement of absorption properties accompanies a greater enhancement of scattering properties, which is reflected in an increase in single scattering albedo (SSA). The enhancement of single scattering albedo due to the morphological effects can reach a factor of 3.75 at 0.67 μm. The asymmetry parameter has a similar yet smaller enhancement. Moreover, the corresponding optical properties of shell-and-core model determined by using Lorenz -Mie solutions are presented for comparison. We found that the optical properties of internally mixed light absorbing carbon aerosol can differ fundamentally from those calculated for the Mie theory shell-and-core model, particularly for thinly coated light absorbing carbon aerosols. Our studies indicate that the complex morphology

Algorithms for radiative transfer simulations for aerosol retrieval

NASA Astrophysics Data System (ADS)

Mukai, Sonoyo; Sano, Itaru; Nakata, Makiko

2012-11-01

Aerosol retrieval work from satellite data, i.e. aerosol remote sensing, is divided into three parts as: satellite data analysis, aerosol modeling and multiple light scattering calculation in the atmosphere model which is called radiative transfer simulation. The aerosol model is compiled from the accumulated measurements during more than ten years provided with the world wide aerosol monitoring network (AERONET). The radiative transfer simulations take Rayleigh scattering by molecules and Mie scattering by aerosols in the atmosphere, and reflection by the Earth surface into account. Thus the aerosol properties are estimated by comparing satellite measurements with the numerical values of radiation simulations in the Earth-atmosphere-surface model. It is reasonable to consider that the precise simulation of multiple light-scattering processes is necessary, and needs a long computational time especially in an optically thick atmosphere model. Therefore efficient algorithms for radiative transfer problems are indispensable to retrieve aerosols from space.

New approaches to quantifying aerosol influence on the cloud radiative effect

DOE PAGES

Feingold, Graham; McComiskey, Allison; Yamaguchi, Takanobu; ...

2016-02-01

The topic of cloud radiative forcing associated with the atmospheric aerosol has been the focus of intense scrutiny for decades. The enormity of the problem is reflected in the need to understand aspects such as aerosol composition, optical properties, cloud condensation, and ice nucleation potential, along with the global distribution of these properties, controlled by emissions, transport, transformation, and sinks. Equally daunting is that clouds themselves are complex, turbulent, microphysical entities and, by their very nature, ephemeral and hard to predict. Atmospheric general circulation models represent aerosol–cloud interactions at ever-increasing levels of detail, but these models lack the resolution tomore » represent clouds and aerosol–cloud interactions adequately. There is a dearth of observational constraints on aerosol–cloud interactions. In this paper, we develop a conceptual approach to systematically constrain the aerosol–cloud radiative effect in shallow clouds through a combination of routine process modeling and satellite and surface-based shortwave radiation measurements. Finally, we heed the call to merge Darwinian and Newtonian strategies by balancing microphysical detail with scaling and emergent properties of the aerosol–cloud radiation system.« less

Measurement-based estimates of direct radiative effects of absorbing aerosols above clouds

NASA Astrophysics Data System (ADS)

Feng, Nan; Christopher, Sundar A.

2015-07-01

The elevated layers of absorbing smoke aerosols from western African (e.g., Gabon and Congo) biomass burning activities have been frequently observed above low-level stratocumulus clouds off the African coast, which presents an excellent natural laboratory for studying the effects of aerosols above clouds (AAC) on regional energy balance in tropical and subtropical environments. Using spatially and temporally collocated Moderate Resolution Imaging Spectroradiometer, Ozone Monitoring Instrument (OMI), and Clouds and the Earth's Radiant Energy System data sets, the top-of-atmosphere shortwave aerosol direct shortwave radiative effects (ARE) of absorbing aerosols above low-level water clouds in the southeast Atlantic Ocean was examined in this study. The regional averaged instantaneous ARE has been estimated to be 36.7 ± 20.5 Wm-2 (regional mean ± standard deviation) along with a mean positive OMI Aerosol Index at 1.3 in August 2006 based on multisensors measurements. The highest magnitude of instantaneous ARE can even reach 138.2 Wm-2. We assess that the 660 nm cloud optical depth (COD) values of 8-12 is the critical value above (below) which aerosol absorption (scattering) effect dominates and further produces positive (negative) ARE values. The results further show that ARE values are more sensitive to aerosols above lower COD values than cases for higher COD values. This is among the first studies to provide quantitative estimates of shortwave ARE due to AAC events from an observational perspective.

Total ozone column, aerosol optical depth and precipitable water effects on solar erythemal ultraviolet radiation recorded in Malta.

NASA Astrophysics Data System (ADS)

Bilbao, Julia; Román, Roberto; Yousif, Charles; Mateos, David; Miguel, Argimiro

2013-04-01

The Universities of Malta and Valladolid (Spain) developed a measurement campaign, which took place in the Institute for Energy Technology in Marsaxlokk (Southern Malta) between May and October 2012, and it was supported by the Spanish government through the Project titled "Measurement campaign about Solar Radiation, Ozone, and Aerosol in the Mediterranean area" (with reference CGL2010-12140-E). This campaign provided the first ground-based measurements in Malta of erythemal radiation and UV index, which indicate the effectiveness of the sun exposure to produce sunburn on human skin. A wide variety of instruments was involved in the campaign, providing a complete atmospheric characterization. Data of erythemal radiation and UV index (from UVB-1 pyranometer), total shortwave radiaton (global and diffuse components from CM-6B pyranometers), and total ozone column, aerosol optical thickness, and precitable water column (from a Microtops-II sunphotometer) were available in the campaign. Ground-based and satellite instruments were used in the analysis, and several intercomparisons were carried out to validate remote sensing data. OMI, GOME, GOME-2, and MODIS instruments, which provide data of ozone, aerosol load and optical properties, were used to this end. The effects on solar radiation, ultraviolet and total shortwave ranges, of total ozone column, aerosol optical thickness and precipitable water column were obtained using radiation measurements at different fixed solar zenith angles. The empirical results shown a determinant role of the solar position, a negligible effect of ozone on total shortwave radiation, and a stronger attenuation provided by aerosol particles in the erythemal radiation. A variety of aerosol types from different sources (desert dust, biomass burning, continental, and maritime) reach Malta, in this campaign several dust events from the Sahara desert occurred and were analyzed establishing the air mass back-trajectories ending at Malta at

Aerosol Radiative Forcing over North India during Pre-Monsoon Season using WRF-Chem

NASA Astrophysics Data System (ADS)

Misra, A.; Kumar, K.; Michael, M.; Tripathi, S. N.

2013-12-01

Study of aerosols is important for a fair understanding of the Earth climate system. This requires knowledge of the physical, chemical, optical, and morphological properties of aerosols. Aerosol radiative forcing provides information on the effect of aerosols on the Earth radiation budget. Radiative forcing estimates using model data provide an opportunity to examine the contribution of individual aerosol species to overall radiative forcing. We have used Weather Research and Forecast with Online Chemistry (WRF-Chem) derived aerosol concentration data to compute aerosol radiative forcing over north India during pre-monsoon season of 2008, 2009, and 2010. WRF-Chem derived mass concentrations are converted to number concentrations using standard procedure. Optical Properties of Aerosol and Cloud (OPAC) software package is used to compute extinction and scattering coefficients, and asymmetry parameter. Computations are performed at different altitudes and the obtained values are integrated to get the column optical properties. Santa Barbara Discrete Ordinate Radiative Transfer (SBDART) model is used to calculate the radiative forcing at surface and top-of-atmosphere. Higher values of aerosol radiative forcing are observed over desert region in western Indian state of Rajasthan, and Punjab of Pakistan. Contribution of individual aerosol species to atmospheric radiative forcing is also assessed. Dust radiative forcing is high over western India. Radiative forcing due to BC and water-soluble (WASO) aerosols are higher over north-west Indian states of Punjab and Haryana, and the Indo-Gangetic Basin. A pool of high WASO optical depth and radiative forcing is observed over the Indo-Bangladesh border. The findings of aerosol optical depth and radiative forcing are consistent with the geography and prevailing aerosol climatology of various regions. Heating rate profiles due to total aerosols and only due to BC have been evaluated at selected stations in north India. They show

Assessment of the first indirect radiative effect of ammonium-sulfate-nitrate aerosols in East Asia

NASA Astrophysics Data System (ADS)

Han, Xiao; Zhang, Meigen; Skorokhod, Andrei

2017-11-01

A physically based cloud nucleation parameterization was introduced into an optical properties/radiative transfer module incorporated with the off-line air quality modeling system Regional Atmospheric Modeling System (RAMS)-Models-3 Community Multi Scale Air Quality (CMAQ) to investigate the distribution features of the first indirect radiative effects of sulfate, nitrate, and ammonium-sulfate-nitrate (ASN) over East Asia for the years of 2005, 2010, and 2013. The relationship between aerosol particles and cloud droplet number concentration could be properly described by this parameterization because the simulated cloud fraction and cloud liquid water path were generally reliable compared with Moderate Resolution Imaging Spectroradiometer (MODIS) retrieved data. Simulation results showed that the strong effect of indirect forcing was mainly concentrated in Southeast China, the East China Sea, the Yellow Sea, and the Sea of Japan. The highest indirect radiative forcing of ASN reached -3.47 W m-2 over Southeast China and was obviously larger than the global mean of the indirect forcing of all anthropogenic aerosols. In addition, sulfate provided about half of the contribution to the ASN indirect forcing effect. However, the effect caused by nitrate was weak because the mass burden of nitrate was very low during summer, whereas the cloud fraction was the highest. The analysis indicated that even though the interannual variation of indirect forcing magnitude generally followed the trend of aerosol mass burden from 2005 to 2013, the cloud fraction was an important factor that determined the distribution pattern of indirect forcing. The heaviest aerosol loading in North China did not cause a strong radiative effect because of the low cloud fraction over this region.

Investigation of short-term effective radiative forcing of fire aerosols over North America using nudged hindcast ensembles

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Yawen; Zhang, Kai; Qian, Yun

Aerosols from fire emissions can potentially have large impact on clouds and radiation. However, fire aerosol sources are often intermittent, and their effect on weather and climate is difficult to quantify. Here we investigated the short-term effective radiative forcing of fire aerosols using the global aerosol–climate model Community Atmosphere Model version 5 (CAM5). Different from previous studies, we used nudged hindcast ensembles to quantify the forcing uncertainty due to the chaotic response to small perturbations in the atmosphere state. Daily mean emissions from three fire inventories were used to consider the uncertainty in emission strength and injection heights. The simulated aerosolmore » optical depth (AOD) and mass concentrations were evaluated against in situ measurements and reanalysis data. Overall, the results show the model has reasonably good predicting skills. Short (10-day) nudged ensemble simulations were then performed with and without fire emissions to estimate the effective radiative forcing. Results show fire aerosols have large effects on both liquid and ice clouds over the two selected regions in April 2009. Ensemble mean results show strong negative shortwave cloud radiative effect (SCRE) over almost the entirety of southern Mexico, with a 10-day regional mean value of –3.0 W m –2. Over the central US, the SCRE is positive in the north but negative in the south, and the regional mean SCRE is small (–0.56 W m –2). For the 10-day average, we found a large ensemble spread of regional mean shortwave cloud radiative effect over southern Mexico (15.6 % of the corresponding ensemble mean) and the central US (64.3 %), despite the regional mean AOD time series being almost indistinguishable during the 10-day period. Moreover, the ensemble spread is much larger when using daily averages instead of 10-day averages. In conclusion, this demonstrates the importance of using a large ensemble of simulations to estimate the short

Investigation of short-term effective radiative forcing of fire aerosols over North America using nudged hindcast ensembles

DOE PAGES

Liu, Yawen; Zhang, Kai; Qian, Yun; ...

2018-01-03

Aerosols from fire emissions can potentially have large impact on clouds and radiation. However, fire aerosol sources are often intermittent, and their effect on weather and climate is difficult to quantify. Here we investigated the short-term effective radiative forcing of fire aerosols using the global aerosol–climate model Community Atmosphere Model version 5 (CAM5). Different from previous studies, we used nudged hindcast ensembles to quantify the forcing uncertainty due to the chaotic response to small perturbations in the atmosphere state. Daily mean emissions from three fire inventories were used to consider the uncertainty in emission strength and injection heights. The simulated aerosolmore » optical depth (AOD) and mass concentrations were evaluated against in situ measurements and reanalysis data. Overall, the results show the model has reasonably good predicting skills. Short (10-day) nudged ensemble simulations were then performed with and without fire emissions to estimate the effective radiative forcing. Results show fire aerosols have large effects on both liquid and ice clouds over the two selected regions in April 2009. Ensemble mean results show strong negative shortwave cloud radiative effect (SCRE) over almost the entirety of southern Mexico, with a 10-day regional mean value of –3.0 W m –2. Over the central US, the SCRE is positive in the north but negative in the south, and the regional mean SCRE is small (–0.56 W m –2). For the 10-day average, we found a large ensemble spread of regional mean shortwave cloud radiative effect over southern Mexico (15.6 % of the corresponding ensemble mean) and the central US (64.3 %), despite the regional mean AOD time series being almost indistinguishable during the 10-day period. Moreover, the ensemble spread is much larger when using daily averages instead of 10-day averages. In conclusion, this demonstrates the importance of using a large ensemble of simulations to estimate the short

Does temperature nudging overwhelm aerosol radiative ...

EPA Pesticide Factsheets

For over two decades, data assimilation (popularly known as nudging) methods have been used for improving regional weather and climate simulations by reducing model biases in meteorological parameters and processes. Similar practice is also popular in many regional integrated meteorology-air quality models that include aerosol direct and indirect effects. However in such multi-modeling systems, temperature changes due to nudging can compete with temperature changes induced by radiatively active & hygroscopic short-lived tracers leading to interesting dilemmas: From weather and climate prediction’s (retrospective or future) point of view when nudging is continuously applied, is there any real added benefit of using such complex and computationally expensive regional integrated modeling systems? What are the relative sizes of these two competing forces? To address these intriguing questions, we convert temperature changes due to nudging into radiative fluxes (referred to as the pseudo radiative forcing, PRF) at the surface and troposphere, and compare the net PRF with the reported aerosol radiative forcing. Results indicate that the PRF at surface dominates PRF at top of the atmosphere (i.e., the net). Also, the net PRF is about 2-4 times larger than estimated aerosol radiative forcing at regional scales while it is significantly larger at local scales. These results also show large surface forcing errors at many polluted urban sites. Thus, operational c

3D Cloud Radiative Effects on Aerosol Optical Thickness Retrievals in Cumulus Cloud Fields in the Biomass Burning Region in Brazil

NASA Technical Reports Server (NTRS)

Wen, Guo-Yong; Marshak, Alexander; Cahalan, Robert F.

2004-01-01

Aerosol amount in clear regions of a cloudy atmosphere is a critical parameter in studying the interaction between aerosols and clouds. Since the global cloud cover is about 50%, cloudy scenes are often encountered in any satellite images. Aerosols are more or less transparent, while clouds are extremely reflective in the visible spectrum of solar radiation. The radiative transfer in clear-cloudy condition is highly three- dimensional (3D). This paper focuses on estimating the 3D effects on aerosol optical thickness retrievals using Monte Carlo simulations. An ASTER image of cumulus cloud fields in the biomass burning region in Brazil is simulated in this study. The MODIS products (i-e., cloud optical thickness, particle effective radius, cloud top pressure, surface reflectance, etc.) are used to construct the cloud property and surface reflectance fields. To estimate the cloud 3-D effects, we assume a plane-parallel stratification of aerosol properties in the 60 km x 60 km ASTER image. The simulated solar radiation at the top of the atmosphere is compared with plane-parallel calculations. Furthermore, the 3D cloud radiative effects on aerosol optical thickness retrieval are estimated.

Challenges in constraining anthropogenic aerosol effects on cloud radiative forcing using present-day spatiotemporal variability.

PubMed

Ghan, Steven; Wang, Minghuai; Zhang, Shipeng; Ferrachat, Sylvaine; Gettelman, Andrew; Griesfeller, Jan; Kipling, Zak; Lohmann, Ulrike; Morrison, Hugh; Neubauer, David; Partridge, Daniel G; Stier, Philip; Takemura, Toshihiko; Wang, Hailong; Zhang, Kai

2016-05-24

A large number of processes are involved in the chain from emissions of aerosol precursor gases and primary particles to impacts on cloud radiative forcing. Those processes are manifest in a number of relationships that can be expressed as factors dlnX/dlnY driving aerosol effects on cloud radiative forcing. These factors include the relationships between cloud condensation nuclei (CCN) concentration and emissions, droplet number and CCN concentration, cloud fraction and droplet number, cloud optical depth and droplet number, and cloud radiative forcing and cloud optical depth. The relationship between cloud optical depth and droplet number can be further decomposed into the sum of two terms involving the relationship of droplet effective radius and cloud liquid water path with droplet number. These relationships can be constrained using observations of recent spatial and temporal variability of these quantities. However, we are most interested in the radiative forcing since the preindustrial era. Because few relevant measurements are available from that era, relationships from recent variability have been assumed to be applicable to the preindustrial to present-day change. Our analysis of Aerosol Comparisons between Observations and Models (AeroCom) model simulations suggests that estimates of relationships from recent variability are poor constraints on relationships from anthropogenic change for some terms, with even the sign of some relationships differing in many regions. Proxies connecting recent spatial/temporal variability to anthropogenic change, or sustained measurements in regions where emissions have changed, are needed to constrain estimates of anthropogenic aerosol impacts on cloud radiative forcing.

Challenges in constraining anthropogenic aerosol effects on cloud radiative forcing using present-day spatiotemporal variability

PubMed Central

Ghan, Steven; Wang, Minghuai; Zhang, Shipeng; Ferrachat, Sylvaine; Gettelman, Andrew; Griesfeller, Jan; Kipling, Zak; Lohmann, Ulrike; Morrison, Hugh; Neubauer, David; Partridge, Daniel G.; Stier, Philip; Takemura, Toshihiko; Wang, Hailong; Zhang, Kai

2016-01-01

A large number of processes are involved in the chain from emissions of aerosol precursor gases and primary particles to impacts on cloud radiative forcing. Those processes are manifest in a number of relationships that can be expressed as factors dlnX/dlnY driving aerosol effects on cloud radiative forcing. These factors include the relationships between cloud condensation nuclei (CCN) concentration and emissions, droplet number and CCN concentration, cloud fraction and droplet number, cloud optical depth and droplet number, and cloud radiative forcing and cloud optical depth. The relationship between cloud optical depth and droplet number can be further decomposed into the sum of two terms involving the relationship of droplet effective radius and cloud liquid water path with droplet number. These relationships can be constrained using observations of recent spatial and temporal variability of these quantities. However, we are most interested in the radiative forcing since the preindustrial era. Because few relevant measurements are available from that era, relationships from recent variability have been assumed to be applicable to the preindustrial to present-day change. Our analysis of Aerosol Comparisons between Observations and Models (AeroCom) model simulations suggests that estimates of relationships from recent variability are poor constraints on relationships from anthropogenic change for some terms, with even the sign of some relationships differing in many regions. Proxies connecting recent spatial/temporal variability to anthropogenic change, or sustained measurements in regions where emissions have changed, are needed to constrain estimates of anthropogenic aerosol impacts on cloud radiative forcing. PMID:26921324

Direct and semi-direct aerosol radiative effect on the Mediterranean climate variability using a coupled regional climate system model

NASA Astrophysics Data System (ADS)

Nabat, Pierre; Somot, Samuel; Mallet, Marc; Sevault, Florence; Chiacchio, Marc; Wild, Martin

2015-02-01

A fully coupled regional climate system model (CNRM-RCSM4) has been used over the Mediterranean region to investigate the direct and semi-direct effects of aerosols, but also their role in the radiation-atmosphere-ocean interactions through multi-annual ensemble simulations (2003-2009) with and without aerosols and ocean-atmosphere coupling. Aerosols have been taken into account in CNRM-RCSM4 through realistic interannual monthly AOD climatologies. An evaluation of the model has been achieved, against various observations for meteorological parameters, and has shown the ability of CNRM-RCSM4 to reproduce the main patterns of the Mediterranean climate despite some biases in sea surface temperature (SST), radiation and cloud cover. The results concerning the aerosol radiative effects show a negative surface forcing on average because of the absorption and scattering of the incident radiation. The SW surface direct effect is on average -20.9 Wm-2 over the Mediterranean Sea, -14.7 Wm-2 over Europe and -19.7 Wm-2 over northern Africa. The LW surface direct effect is weaker as only dust aerosols contribute (+4.8 Wm-2 over northern Africa). This direct effect is partly counterbalanced by a positive semi-direct radiative effect over the Mediterranean Sea (+5.7 Wm-2 on average) and Europe (+5.0 Wm-2) due to changes in cloud cover and atmospheric circulation. The total aerosol effect is consequently negative at the surface and responsible for a decrease in land (on average -0.4 °C over Europe, and -0.5 °C over northern Africa) and sea surface temperature (on average -0.5 °C for the Mediterranean SST). In addition, the latent heat loss is shown to be weaker (-11.0 Wm-2) in the presence of aerosols, resulting in a decrease in specific humidity in the lower troposphere, and a reduction in cloud cover and precipitation. Simulations also indicate that dust aerosols warm the troposphere by absorbing solar radiation, and prevent radiation from reaching the surface, thus

Air pollution and climate response to aerosol direct radiative ...

EPA Pesticide Factsheets

Decadal hemispheric Weather Research and Forecast-Community Multiscale Air Quality simulations from 1990 to 2010 were conducted to examine the meteorology and air quality responses to the aerosol direct radiative effects. The model's performance for the simulation of hourly surface temperature, relative humidity, wind speed, and direction was evaluated through comparison with observations from NOAA's National Climatic Data Center Integrated Surface Data. The inclusion of aerosol direct radiative effects improves the model's ability to reproduce the trend in daytime temperature range which over the past two decades was increasing in eastern China but decreasing in eastern U.S. and Europe. Trends and spatial and diurnal variations of the surface-level gaseous and particle concentrations to the aerosol direct effect were analyzed. The inclusion of aerosol direct radiative effects was found to increase the surface-level concentrations of SO2, NO2, O3, SO42−, NO3−, and particulate matter 2.5 in eastern China, eastern U.S., and Europe by 1.5–2.1%, 1–1.5%, 0.1–0.3%, 1.6–2.3%, 3.5–10.0%, and 2.2–3.2%, respectively, on average over the entire 21 year period. However, greater impacts are noted during polluted days with increases of 7.6–10.6%, 6.2–6.7%, 2.0–3.0%, 7.8–9.5%, 11.1–18.6%, and 7.2–10.1%, respectively. Due to the aerosol direct radiative effects, stabilizing of the atmosphere associated with reduced planetary boundary layer height a

Long-term Satellite Observations of Cloud and Aerosol Radiative Effects Using the (A)ATSR Satellite Data Record

NASA Astrophysics Data System (ADS)

Christensen, M.; McGarragh, G.; Thomas, G.; Povey, A.; Proud, S.; Poulsen, C. A.; Grainger, R. G.

2016-12-01

Radiative forcing by clouds, aerosols, and their interactions constitute some of the largest sources of uncertainties in the climate system (Chapter 7 IPCC, 2013). It is essential to understand the past through examination of long-term satellite observation records to provide insight into the uncertainty characteristics of these radiative forcers. As part of the ESA CCI (Climate Change Initiative) we have recently implemented a broadband radiative flux algorithm (known as BUGSrad) into the Optimal Retrieval for Aerosol and Cloud (ORAC) scheme. ORAC achieves radiative consistency of its aerosol and cloud products through an optimal estimation scheme and is highly versatile, enabling retrievals for numerous satellite sensors: ATSR, MODIS, VIIRS, AVHRR, SLSTR, SEVIRI, and AHI. An analysis of the 17-year well-calibrated Along Track Scanning Radiometer (ATSR) data is used to quantify trends in cloud and aerosol radiative effects over a wide range of spatiotemporal scales. The El Niño Southern Oscillation stands out as the largest contributing mode of variability to the radiative energy balance (long wave and shortwave fluxes) at the top of the atmosphere. Furthermore, trends in planetary albedo show substantial decreases across the Arctic Ocean (likely due to the melting of sea ice and snow) and modest increases in regions dominated by stratocumulus (e.g., off the coast of California) through notable increases in cloud fraction and liquid water path. Finally, changes in volcanic activity and biomass burning aerosol over this period show sizeable radiative forcing impacts at local-scales. We will demonstrate that radiative forcing from aerosols and clouds have played a significant role in the identified key climate processes using 17 years of satellite observational data.

Parameterization of clear-sky surface irradiance and its implications for estimation of aerosol direct radiative effect and aerosol optical depth

PubMed Central

Xia, Xiangao

2015-01-01

Aerosols impact clear-sky surface irradiance () through the effects of scattering and absorption. Linear or nonlinear relationships between aerosol optical depth (τa) and have been established to describe the aerosol direct radiative effect on (ADRE). However, considerable uncertainties remain associated with ADRE due to the incorrect estimation of (τa in the absence of aerosols). Based on data from the Aerosol Robotic Network, the effects of τa, water vapor content (w) and the cosine of the solar zenith angle (μ) on are thoroughly considered, leading to an effective parameterization of as a nonlinear function of these three quantities. The parameterization is proven able to estimate with a mean bias error of 0.32 W m−2, which is one order of magnitude smaller than that derived using earlier linear or nonlinear functions. Applications of this new parameterization to estimate τa from , or vice versa, show that the root-mean-square errors were 0.08 and 10.0 Wm−2, respectively. Therefore, this study establishes a straightforward method to derive from τa or estimate τa from measurements if water vapor measurements are available. PMID:26395310

Physical and Optical/Radiative Properties of Arctic Aerosols: Potential Effects on Arctic Climate

NASA Technical Reports Server (NTRS)

Pueschel, R. F.; Kinne, S. A.; Gore, Warren J. (Technical Monitor)

1994-01-01

We have determined the abundance of light-scattering sulfuric acid (H2SO4/H2O) and light-absorbing black carbon aerosol (BCA) in Spring 1992 in the Arctic atmosphere by airborne in situ sampling with impactors, and measured particle sizes and morphologies by scanning electron microscopy. The mass of BCA in the Arctic troposphere is one percent of the total aerosol, reduced to one part in 104 in the stratosphere. A Mie algorithm permits the calculation of the optical properties of the various aerosol components, and an algorithm developed by Ackerman and Toon and modified to serve our needs lets us calculate the optical effects of the black carbon aerosol that is mixed internally with the sulfuric acid aerosol. It follows that the effect of internally-mixed BCA on the aerosol scattering and absorption properties depends on its location within the droplet. BCA concentrated near the droplet surface has a greater effect on absorption of solar radiation than does the same amount of BCA located near its center. Single scatter albedos of the combined system are omega(sub 0)=1.0 in the post-Pinatubo Arctic stratosphere, and as low as 0.94 in the troposphere. The aerosol has the potential to regionally warm the Arctic earth-atmosphere system, because of the high surface albedo of the snow-covered Arctic.

Impacts of Aerosol Direct Effects on the South Asian climate: Assessment of Radiative Feedback Processes Using Model Simulations and Satellite/surface Measurements

NASA Astrophysics Data System (ADS)

Wang, S.; Gautam, R.; Lau, W. K.; Tsay, S.; Sun, W.; Kim, K.; Chern, J.; Colarco, P. R.; Hsu, N. C.; Lin, N.

2011-12-01

Current assessment of aerosol radiative effect is hindered by our incomplete knowledge of aerosol optical properties, especially absorption, and our current inability to quantify physical and microphysical processes. In this research, we investigate direct aerosol radiative effect over heavy aerosol loading areas (e.g., Indo-Gangetic Plains, South/East Asia) and its feedbacks on the South Asian climate during the pre-monsoon season (March-June) using the Purdue Regional Climate Model (PRCM) with prescribed aerosol data derived by the NASA Goddard Earth Observing System Model (GEOS-5). Our modeling domain covers South and East Asia (60-140E and 0-50N) with spatial resolutions of 45 km in horizontal and 28 layers in vertical. The model is integrated from 15 February to 30 June 2008 continuously without nudging (i.e., only forced by initial/boundary conditions). Two numerical experiments are conducted with and without the aerosol-radiation effects. Both simulations are successful in reproducing the synoptic patterns on seasonal-to-interannual time scales and capturing a pre-monsoon feature of the northward rainfall propagation over Indian region in early June which shown in Tropical Rainfall Measuring Mission (TRMM) observation. Preliminary result suggests aerosol-radiation interactions mainly alter surface-atmosphere energetics and further result in an adjustment of the vertical temperature distribution in lower atmosphere (below 700 hPa). The modifications of temperature and associated rainfall and circulation feedbacks on the regional climate will be discussed in the presentation. In addition to modeling study, we will also present the most recent results on aerosol properties, regional aerosol absorption, and radiative forcing estimation based on NASA's operational satellite and ground-based remote sensing. Observational results show spatial gradients in aerosol loading and solar absorption accounting over Indo-Gangetic Plains during the pre-monsoon season. The

Application of Satellite and Ground-based Data to Investigate the UV Radiative Effects of Australian Aerosols

NASA Technical Reports Server (NTRS)

Kalashnikova, Olga V.; Mills, Franklin P.; Eldering, Annmarie; Anderson, Don

2007-01-01

An understanding of the effect of aerosols on biologically- and photochemically-active UV radiation reaching the Earth's surface is important for many ongoing climate, biophysical, and air pollution studies. In particular, estimates of the UV characteristics of the most common Australian aerosols will be valuable inputs to UV Index forecasts, air quality studies, and assessments of the impact of regional environmental changes. By analyzing climatological distributions of Australian aerosols we have identified sites where co-located ground-based UV-B and ozone measurements were available during episodes of relatively high aerosol activity. Since at least June 2003, surface UV global irradiance spectra (285-450 nm) have been measured routinely at Darwin and Alice Springs in Australia by the Australian Bureau of Meteorology (BoM). Using colocated sunphotometer measurements at Darwin and Alice Springs, we identified several episodes of relatively high aerosol activity. Aerosol air mass types were analyzed from sunphotometer-derived angstrom parameter, MODIS fire maps and MISR aerosol property retrievals. To assess aerosol effects we compared the measured UV irradiances for aerosol-loaded and clear-sky conditions with each other and with irradiances simulated using the libRadtran radiative transfer model for aerosol-free conditions. We found that for otherwise similar atmospheric conditions, smoke aerosols over Darwin reduced the surface UV irradiance by as much as 40-50% at 290-300 nm and 20-25% at 320-400 nm near active fires (aerosol optical depth, AOD, at 500 nm approximately equal to 0.6). Downwind of fires, the smoke aerosols over Darwin reduced the surface irradiance by 15-25% at 290-300 nm and approximately 10% at 320-350 nm (AOD at 500 nm approximately equal to 0.2). The effect of smoke increased with decrease of wavel strongest in the UV-B. The aerosol attenuation factors calculated for the selected cases suggest smoke over Darwin has an effect on surface 340

Direct Aerosol Radiative Forcing: Calculations and Measurements from the Tropospheric

NASA Technical Reports Server (NTRS)

Russell, P. B.; Hignett, P.; Stowe, L. L.; Livingston, J. M.; Kinne, S.; Wong, J.; Chan, K. Roland (Technical Monitor)

1997-01-01

Radiative forcing is defined as the change in the net (downwelling minus upwelling) radiative flux at a given level in the atmosphere. This net flux is the radiative power density available to drive climatic processes in the earth-atmosphere system below that level. Recent research shows that radiative forcing by aerosol particles is a major source of uncertainty in climate predictions. To reduce those uncertainties, TARFOX was designed to determine direct (cloud-free) radiative forcing by the aerosols in one of the world's major industrial pollution plumes--that flowing from the east coast of the US over the Atlantic Ocean. TARFOX measured a variety of aerosol radiative effects (including direct forcing) while simultaneously measuring the chemical, physical, and optical properties of the aerosol particles causing those effects. The resulting data sets permit a wide variety of tests of the consistency, or closure, among the measurements and the models that link them. Because climate predictions use the same or similar model components, closure tests help to assess and reduce prediction uncertainties. In this work we use the TARFOX-determined aerosol, gas, and surface properties to compute radiative forcing for a variety of aerosol episodes, with inadvisable optical depths ranging from 0.07 to 0.6. We calculate forcing by several techniques with varying degrees of sophistication, in part to test the range of applicability of simplified techniques--which are often the only ones feasible in climate predictions by general circulation models (GCMs). We then compare computed forcing to that determined from: (1) Upwelling and downwelling fluxes (0.3-0.7 mm and 0.7-3.0 mm) measured by radiometers on the UK MRF C-130. and (2) Daily average cloud-free absorbed solar and emitted thermal radiative flux at the top of the atmosphere derived from the AVHRR radiometer on the NOAA- 14 satellite. The calculations and measurements all yield aerosol direct radiative forcing in the

Investigation of Trends in Aerosol Direct Radiative Effects over North America Using a Coupled Meteorology-Chemistry Model

EPA Science Inventory

A comprehensive investigation of the processes regulating tropospheric aerosol distributions, their optical properties, and their radiative effects in conjunction with verification of their simulated radiative effects for past conditions relative to measurements is needed in orde...

Aerosol polarization effects on atmospheric correction and aerosol retrievals in ocean color remote sensing.

PubMed

Wang, Menghua

2006-12-10

The current ocean color data processing system for the Sea-viewing Wide Field-of-View Sensor (SeaWiFS) and the moderate resolution imaging spectroradiometer (MODIS) uses the Rayleigh lookup tables that were generated using the vector radiative transfer theory with inclusion of the polarization effects. The polarization effects, however, are not accounted for in the aerosol lookup tables for the ocean color data processing. I describe a study of the aerosol polarization effects on the atmospheric correction and aerosol retrieval algorithms in the ocean color remote sensing. Using an efficient method for the multiple vector radiative transfer computations, aerosol lookup tables that include polarization effects are generated. Simulations have been carried out to evaluate the aerosol polarization effects on the derived ocean color and aerosol products for all possible solar-sensor geometries and the various aerosol optical properties. Furthermore, the new aerosol lookup tables have been implemented in the SeaWiFS data processing system and extensively tested and evaluated with SeaWiFS regional and global measurements. Results show that in open oceans (maritime environment), the aerosol polarization effects on the ocean color and aerosol products are usually negligible, while there are some noticeable effects on the derived products in the coastal regions with nonmaritime aerosols.

Aerosol radiative forcing from GEO satellite data over land surfaces

NASA Astrophysics Data System (ADS)

Costa, Maria J.; Silva, Ana M.

2005-10-01

Aerosols direct and indirect effects on the Earth's climate are widely recognized but have yet to be adequately quantified. Difficulties arise due to the very high spatial and temporal variability of aerosols, which is a major cause of uncertainties in radiative forcing studies. The effective monitoring of the global aerosol distribution is only made possible by satellite monitoring and this is the reason why the interest in aerosol observations from satellite passive radiometers is steadily increasing. From the point of view of the study of land surfaces, the atmosphere with its constituents represents an obscurant whose effects should be as much as possible eliminated, being this process sometimes referred to as atmospheric correction. In absence of clouds and using spectral intervals where gas absorption can be avoided to a great extent, only the aerosol effect remains to be corrected. The monitoring of the aerosol particles present in the atmosphere is then crucial to succeed in doing an accurate atmospheric correction, otherwise the surface properties may be inadequately characterised. However, the atmospheric correction over land surfaces turns out to be a difficult task since surface reflection competes with the atmospheric component of the signal. On the other hand, a single mean pre-established aerosol characterisation would not be sufficient for this purpose due to very high spatial and temporal variability of aerosols and their unpredictability, especially what concerns particulary intense "events" such as biomass burning and forest fires, desert dust episodes and volcanic eruptions. In this context, an operational methodology has been developed at the University of Evora - Evora Geophysics Centre (CGE), in the framework of the Satellite Application Facility for Land Surface Analysis - Land SAF, to derive an Aerosol Product from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) data, flying on the Geostationary (GEO) satellite system Meteosat-8

A global modeling study on carbonaceous aerosol microphysical characteristics and radiative forcing

NASA Astrophysics Data System (ADS)

Bauer, S. E.; Menon, S.; Koch, D.; Bond, T. C.; Tsigaridis, K.

2010-02-01

Recently, attention has been drawn towards black carbon aerosols as a short-term climate warming mitigation candidate. However the global and regional impacts of the direct, cloud-indirect and semi-direct forcing effects are highly uncertain, due to the complex nature of aerosol evolution and the way that mixed, aged aerosols interact with clouds and radiation. A detailed aerosol microphysical scheme, MATRIX, embedded within the GISS climate model is used in this study to present a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative forcing. Our best estimate for net direct and indirect aerosol radiative forcing between 1750 and 2000 is -0.56 W/m2. However, the direct and indirect aerosol effects are quite sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative forcing can vary between -0.32 to -0.75 W/m2 depending on these carbonaceous particle properties at emission. Assuming that sulfates, nitrates and secondary organics form a coating around a black carbon core, rather than forming a uniformly mixed particle, changes the overall net aerosol radiative forcing from negative to positive. Taking into account internally mixed black carbon particles let us simulate correct aerosol absorption. Black carbon absorption is amplified by sulfate and nitrate coatings, but even more strongly by organic coatings. Black carbon mitigation scenarios generally showed reduced radiative forcing when sources with a large proportion of black carbon, such as diesel, are reduced; however reducing sources with a larger organic carbon component as well, such as bio-fuels, does not necessarily lead to climate benefits.

Direct Radiative Impacts of Central American Biomass Burning Smoke Aerosols: Analysis from a Coupled Aerosol-Radiation-Meteorology Model RAMS-AROMA

NASA Astrophysics Data System (ADS)

Wang, J.; Christopher, S. A.; Nair, U. S.; Reid, J. S.; Prins, E. M.

2005-12-01

Considerable efforts including various field experiments have been carried out in the last decade for studying the regional climatic impact of smoke aerosols produced by biomass burning activities in Africa and South America. In contrast, only few investigations have been conducted for Central American Biomass Burning (CABB) region. Using a coupled aerosol-radiation-meteorology model called RAMS-AROMA together with various ground-based observations, we present a comprehensive analysis of the smoke direct radiative impacts on the surface energy budget, boundary layer evolution, and e precipitation process during the CABB events in Spring 2003. Quantitative estimates are also made regarding the transboundary carbon mass to the U.S. in the form of smoke particles. Buult upon the Regional Atmospheric Modeling System (RAMS) mesoscale model, the RAMS AROMA has several features including Assimilation and Radiation Online Modeling of Aerosols (AROMA) algorithms. The model simulates smoke transport by using hourly smoke emission inventory from the Fire Locating and Modeling of Burning Emissions (FLAMBE) geostationary satellite database. It explicitly considers the smoke effects on the radiative transfer at each model time step and model grid, thereby coupling the dynamical processes and aerosol transport. Comparison with ground-based observation show that the simulation realistically captured the smoke transport timeline and distribution from daily to hourly scales. The effects of smoke radiative extinction on the decrease of 2m air temperature (2mT), diurnal temperature range (DTR), and boundary layer height over the land surface are also quantified. Warming due to smoke absorption of solar radiation can be found in the lower troposphere over the ocean, but not near the underlying land surface. The increase of boundary layer stability produces a positive feedback where more smoke particles are trapped in the lower boundary layer. These changes in temperature, surface

A multi-satellite analysis of the direct radiative effects of absorbing aerosols above clouds

NASA Astrophysics Data System (ADS)

Chang, Y. Y.; Christopher, S. A.

2015-12-01

Radiative effects of absorbing aerosols above liquid water clouds in the southeast Atlantic as a function of fire sources are investigated using A-Train data coupled with the Visible Infrared Imaging Radiometer Suite (VIIRS) onboard Suomi National Polar-orbiting Partnership (Suomi NPP). Both the VIIRS Active Fire product and the Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) Thermal Anomalies product (MYD14) are used to identify the biomass burning fire origin in southern Africa. The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) are used to assess the aerosol type, aerosol altitude, and cloud altitude. We use back trajectory information, wind data, and the Fire Locating and Modeling of Burning Emissions (FLAMBE) product to infer the transportation of aerosols from the fire source to the CALIOP swath in the southeast Atlantic during austral winter.

"Investigation of Trends in Aerosol Direct Radiative Effects over North America Using a Coupled Meteorology-Chemistry Model"

EPA Science Inventory

While aerosol radiative effects have been recognized as some of the largest sources of uncertainty among the forcers of climate change, there has been little effort devoted to verification of the spatial and temporal variability of the magnitude and directionality of aerosol radi...

Observationally constrained estimates of carbonaceous aerosol radiative forcing.

PubMed

Chung, Chul E; Ramanathan, V; Decremer, Damien

2012-07-17

Carbonaceous aerosols (CA) emitted by fossil and biomass fuels consist of black carbon (BC), a strong absorber of solar radiation, and organic matter (OM). OM scatters as well as absorbs solar radiation. The absorbing component of OM, which is ignored in most climate models, is referred to as brown carbon (BrC). Model estimates of the global CA radiative forcing range from 0 to 0.7 Wm(-2), to be compared with the Intergovernmental Panel on Climate Change's estimate for the pre-Industrial to the present net radiative forcing of about 1.6 Wm(-2). This study provides a model-independent, observationally based estimate of the CA direct radiative forcing. Ground-based aerosol network data is integrated with field data and satellite-based aerosol observations to provide a decadal (2001 through 2009) global view of the CA optical properties and direct radiative forcing. The estimated global CA direct radiative effect is about 0.75 Wm(-2) (0.5 to 1.0). This study identifies the global importance of BrC, which is shown to contribute about 20% to 550-nm CA solar absorption globally. Because of the inclusion of BrC, the net effect of OM is close to zero and the CA forcing is nearly equal to that of BC. The CA direct radiative forcing is estimated to be about 0.65 (0.5 to about 0.8) Wm(-2), thus comparable to or exceeding that by methane. Caused in part by BrC absorption, CAs have a net warming effect even over open biomass-burning regions in Africa and the Amazon.

Observationally constrained estimates of carbonaceous aerosol radiative forcing

PubMed Central

Chung, Chul E.; Ramanathan, V.; Decremer, Damien

2012-01-01

Carbonaceous aerosols (CA) emitted by fossil and biomass fuels consist of black carbon (BC), a strong absorber of solar radiation, and organic matter (OM). OM scatters as well as absorbs solar radiation. The absorbing component of OM, which is ignored in most climate models, is referred to as brown carbon (BrC). Model estimates of the global CA radiative forcing range from 0 to 0.7 Wm-2, to be compared with the Intergovernmental Panel on Climate Change’s estimate for the pre-Industrial to the present net radiative forcing of about 1.6 Wm-2. This study provides a model-independent, observationally based estimate of the CA direct radiative forcing. Ground-based aerosol network data is integrated with field data and satellite-based aerosol observations to provide a decadal (2001 through 2009) global view of the CA optical properties and direct radiative forcing. The estimated global CA direct radiative effect is about 0.75 Wm-2 (0.5 to 1.0). This study identifies the global importance of BrC, which is shown to contribute about 20% to 550-nm CA solar absorption globally. Because of the inclusion of BrC, the net effect of OM is close to zero and the CA forcing is nearly equal to that of BC. The CA direct radiative forcing is estimated to be about 0.65 (0.5 to about 0.8) Wm-2, thus comparable to or exceeding that by methane. Caused in part by BrC absorption, CAs have a net warming effect even over open biomass-burning regions in Africa and the Amazon. PMID:22753522

Long-term variability of aerosol optical properties and radiative effects in Northern Finland

NASA Astrophysics Data System (ADS)

Lihavainen, Heikki; Hyvärinen, Antti; Asmi, Eija; Hatakka, Juha; Viisanen, Yrjö

2017-04-01

We introduce long term dataset of aerosol scattering and absorption properties and combined aerosol optical properties measured in Pallas Atmosphere-Ecosystem Supersite in Norhern Finland. The station is located 170 km north of the Arctic Circle. The station is affected by both pristine Arctic air masses as well as long transported air pollution from northern Europe. We studied the optical properties of aerosols and their radiative effects in continental and marine air masses, including seasonal cycles and long-term trends. The average (median) scattering coefficient, backscattering fraction, absorption coefficient and single scattering albedo at the wavelength of 550 nm were 7.9 (4.4) 1/Mm, 0.13 (0.12), 0.74 (0.35) 1/Mm and 0.92 (0.93), respectively. We observed clear seasonal cycles in these variables, the scattering coefficient having high values during summer and low in fall, and absorption coefficient having high values during winter and low in fall. We found that the high values of the absorption coefficient and low values of the single scattering albedo were related to continental air masses from lower latitudes. These aerosols can induce an additional effect on the surface albedo and melting of snow. We observed the signal of the Arctic haze in marine (northern) air masses during March and April. The haze increased the value of the absorption coefficient by almost 80% and that of the scattering coefficient by about 50% compared with the annual-average values. We did not observe any long-term trend in the scattering coefficient, while our analysis showed a clear decreasing trend in the backscattering fraction and scattering Ångström exponent during winter. We also observed clear relationship with temperature and aerosol scattering coefficient. We will present also how these different features affects to aerosol direct radiative forcing.

Aerosol Particle Shape and Radiative Coupling in a Three Dimensional Titan GCM

NASA Astrophysics Data System (ADS)

Larson, Erik J.; Toon, O. B.; Friedson, A. J.; West, R. A.

2010-10-01

Understanding the aerosols on Titan is imperative for understanding the atmosphere as a whole. The aerosols affect the albedo, optical depth, as well as heating and cooling rates which in turn affect the circulation on Titan leading to feedback with the aerosol distribution. Correctly representing the aerosols in atmospheric models is crucial to understanding this atmosphere. Friedson et al. (2009, A global climate model of Titan's atmosphere and surface. Planet. SpaceSci. 57, 1931-1949.) produced a three-dimensional model for Titan using the NCAR CAM3 model, to which we coupled the aerosol microphysics model CARMA. We have also made the aerosols produced by CARMA interactive with the radiation code in CAM. We compare simulations with radiatively interactive aerosols with those using a prescribed aerosol radiative effect. Preliminary results show that this model is capable of reproducing the seasonal changes in aerosols on Titan and many of the associated phenomena. For instance, the radiatively interactive aerosols are lofted by winds more in the summer hemisphere than the non-radiatively interactive aerosols, which is necessary to reproduce the observed seasonal cycle of the albedo. We compare simulations using spherical particles to simulations using fractal aggregate particles, which are expected from laboratory and observational data. Fractal particles have higher absorption in the UV, slower fall velocities and faster coagulation rates than equivalent mass spherical particles. We compare model simulations with observational data from the Cassini and Huygens missions.

From nuclear power to coal power: Aerosol-induced health and radiative effects

NASA Astrophysics Data System (ADS)

Mielonen, Tero; Laakso, Anton; Karhunen, Anni; Kokkola, Harri; Partanen, Antti-Ilari; Korhonen, Hannele; Romakkaniemi, Sami; Lehtinen, Kari E. J.

2015-12-01

We have investigated what would be the climate and PM-induced air quality consequences if all nuclear reactors worldwide were closed down and replaced by coal combustion. In a way, this presents a "worst-case scenario" since less polluting energy sources are available. We studied simultaneously the radiative and health effects of coal power emissions using a global 3-D aerosol-climate model (ECHAM-HAMMOZ). This approach allowed us to estimate the effects of a major global energy production change from low carbon source to a high carbon one using detailed spatially resolved population density information. We included the radiative effects of both CO2 and PM2.5 but limited the study of health effects to PM2.5 only. Our results show that the replacement of nuclear power with coal power would have globally caused an average of 150,000 premature deaths per year during the period 2005-2009 with two thirds of them in Europe. For 37 years the aerosol emissions from the additional coal power plants would cool the climate but after that the accumulating CO2 emissions would accelerate the warming of the climate.

Aerosol Absorption Effects in the TOMS UV Algorithm

NASA Technical Reports Server (NTRS)

Torres, O.; Krotkov, N.; Bhartia, P. K.

2004-01-01

The availability of global long-term estimates of surface UV radiation is very important, not only for preventive medicine considerations, but also as an important tool to monitor the effects of the stratospheric ozone recovery expected to occur in the next few decades as a result of the decline of the stratospheric chlorine levels. In addition to the modulating effects of ozone and clouds, aerosols also affect the levels of UV-A and W-B radiation reaching the surface. Oscillations in surface W associated with the effects of aerosol absorption may be comparable in magnitude to variations associated with the stratospheric ozone recovery. Thus, the accurate calculation of surface W radiation requires that both the scattering and absorption effects of tropospheric aerosols be taken into account. Although absorption effects of dust and elevated carbonaceous aerosols are already accounted for using Aerosol Index technique, this approach does not work for urban/industrial aerosols in the planetary boundary layer. The use of the new TOMS long-term global data record on UV aerosol absorption optical depth, can improve the accuracy of TOMS spectral UV products, by properly including the spectral attenuation effects of carbonaceous, urban/industrial and mineral aerosols. The TOMS data set on aerosol properties will be discussed, and results of its use in the TOMS surface W algorithm will be presented.

North Atlantic Aerosol Radiative Effects Based on Satellite Measurements and Aerosol Intensive Properties from TARFOX and ACE-2

NASA Technical Reports Server (NTRS)

Bergstrom, Robert W.; Russell, Philip B.

2000-01-01

We estimate the impact of North Atlantic aerosols on the net shortwave flux at the tropopause by combining maps of satellite-derived aerosol optical depth (AOD) with model aerosol properties. We exclude African dust, primarily by restricting latitudes to 25-60 N. Aerosol properties were determined via column closure analyses in two recent experiments, TARFOX and ACE 2. The analyses use in situ measurements of aerosol composition and air- and ship-borne sunphotometer measurements of AOD spectra. The resulting aerosol model yields computed flux sensitivities (dFlux/dAOD) that agree with measurements by airborne flux radiometers in TARFOX. It has a midvisible single-scattering albedo of 0.9, which is in the range obtained from in situ measurements of aerosol scattering and absorption in both TARFOX and ACE 2. Combining seasonal maps of AVHRR-derived midvisible AOD with the aerosol model yields maps of 24-hour average net radiative flux changes at the tropopause. For cloud-free conditions, results range from -9 W/sq m near the eastern US coastline in the summer to -1 W/sq m in the mid-Atlantic during winter; the regional annual average is -3.5 W/sq m. Using a non- absorbing aerosol model increases these values by about 30%. We estimate the effect of clouds using ISCCP cloud-fraction maps. Because ISCCP midlatitude North Atlantic cloud fractions are relatively large, they greatly reduce the computed aerosol-induced flux changes. For example, the regional annual average decreases from -3.5 W/sq m to -0.8 W/sq m. We compare results to previous model calculations for a variety of aerosol types.

Assessment of cirrus cloud and aerosol radiative effect in South-East Asia by ground-based NASA MPLNET lidar network data and CALIPSO satellite measurements

NASA Astrophysics Data System (ADS)

Lolli, Simone; Campbell, James R.; Lewis, Jasper R.; Welton, Ellsworth J.; Di Girolamo, Paolo; Fatkhuroyan, Fatkhuroyan; Gu, Yu; Marquis, Jared W.

2017-10-01

Aerosol, together with cirrus clouds, play a fundamental role in the earth-atmosphere system radiation budget, especially at tropical latitudes, where the Earth surface coverage by cirrus cloud can easily reach 70%. In this study we evaluate the combined aerosol and cirrus cloud net radiative effects in a wild and barren region like South East Asia. This part of the world is extremely vulnerable to climate change and it is source of important anthropogenic and natural aerosol emissions. The analysis has been carried out by computing cirrus cloud and aerosol net radiative effects through the Fu-Liou-Gu atmospheric radiative transfer model, adequately adapted to input lidar measurements, at surface and top-of-the atmosphere. The aerosol radiative effects were computed respectively using the retrieved lidar extinction from Cloud-Aerosol Lidar with Orthogonal Polarization in 2011 and 2012 and the lidar on-board of Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations for the South East Asia Region (27N-12S, 77E-132E) with 5° x 5° spatial resolution. To assess the cirrus cloud radiative effect, we used the ground-based Micro Pulse Lidar Network measurements at Singapore permanent observational site. Results put in evidence that strong aerosol emission areas are related on average to a net surface cooling. On the contrary, cirrus cloud radiative effect shows a net daytime positive warming of the system earth-atmosphere. This effect is weak over the ocean where the albedo is lower and never counter-balances the net cooling produced by aerosols. The net cooling is stronger in 2011, with an associated reduction in precipitations by the four of the five rain-gauges stations deployed in three regions as Sumatra, Kalimantan and Java with respect to 2012. We can speculate that aerosol emissions may be associated with lower rainfall, however some very important phenomena as El Nino Southern Oscillation , Madden-Julian Oscillation, Monsoon and Indian Dipole are not

Radiative Effects of Carbonaceous and Inorganic Aerosols over California during CalNex and CARES: Observations versus Model Predictions

NASA Astrophysics Data System (ADS)

Vinoj, V.; Fast, J. D.; Liu, Y.

2012-12-01

Aerosols have been identified to be a major contributor to the uncertainty in understanding the present climate. Most of this uncertainty arises due to the lack of knowledge of their micro-physical and chemical properties as well as how to adequately represent their spatial and temporal distributions. Increased process level understanding can be achieved through carefully designed field campaigns and experiments. These measurements can be used to elucidate the aerosol properties, mixing, transport and transformation within the atmosphere and also to validate and improve models that include meteorology-aerosol-chemistry interactions. In the present study, the WRF-Chem model is used to simulate the evolution of carbonaceous and inorganic aerosols and their impact on radiation during May and June of 2010 over California when two field campaigns took place: the California Nexus Experiment (CalNex) and Carbonaceous Aerosol and Radiative Effects Study (CARES). We merged CalNex and CARES data along with data from operational networks such as, California Air Resources Board (CARB's) air quality monitoring network, the Interagency Monitoring of Protected Visual Environments (IMPROVE) network, the AErosol RObotic NETwork (AERONET), and satellites into a common dataset for the Aerosol Modeling Test bed. The resulting combined dataset is used to rigorously evaluate the model simulation of aerosol mass, size distribution, composition, and optical properties needed to understand uncertainties that could affect regional variations in aerosol radiative forcing. The model reproduced many of the diurnal, multi-day, and spatial variations of aerosols as seen in the measurements. However, regionally the performance varied with reasonably good agreement with observations around Los Angeles and Sacramento and poor agreement with observations in the vicinity of Bakersfield (although predictions aloft were much better). Some aerosol species (sulfate and nitrate) were better represented

Aerosols and their Impact on Radiation, Clouds, Precipitation & Severe Weather Events

DOE Office of Scientific and Technical Information (OSTI.GOV)

Li, Zhanqing; Rosenfeld, Daniel; Fan, Jiwen

Aerosols, the tiny particles suspended in the atmosphere, have been in the forefront of environmental and climate change sciences as the primary atmospheric pollutant and external force affecting Earth’s weather and climate. There are two dominant mechanisms by which aerosols affect weather and climate: aerosol-radiation interactions (ARI) and aerosol-cloud interactions (ACI). ARI arises from aerosol scattering and absorption, which alters the radiation budgets of the atmosphere and surface, while ACI is rooted to the fact that aerosols serve as cloud condensation nuclei and ice nuclei. Both ARI and ACI are coupled with atmospheric dynamics to produce a chain of complexmore » interactions with a large range of meteorological variables that influence both weather and climate. Elaborated here are the impacts of aerosols on the radiation budget, clouds (microphysics, structure, and lifetime), precipitation, and severe weather events (lightning, thunderstorms, hail, and tornados). Depending on environmental variables and aerosol properties, the effects can be both positive and negative, posing the largest uncertainties in the external forcing of the climate system. This has considerably hindered our ability in projecting future climate changes and in doing accurate numerical weather predictions.« less

Historical anthropogenic radiative forcing of changes in biogenic secondary aerosol

NASA Astrophysics Data System (ADS)

Acosta Navarro, Juan; D'Andrea, Stephen; Pierce, Jeffrey; Ekman, Annica; Struthers, Hamish; Zorita, Eduardo; Guenther, Alex; Arneth, Almut; Smolander, Sampo; Kaplan, Jed; Farina, Salvatore; Scott, Catherine; Rap, Alexandru; Farmer, Delphine; Spracklen, Domink; Riipinen, Ilona

2016-04-01

Human activities have lead to changes in the energy balance of the Earth and the global climate. Changes in atmospheric aerosols are the second largest contributor to climate change after greenhouse gases since 1750 A.D. Land-use practices and other environmental drivers have caused changes in the emission of biogenic volatile organic compounds (BVOCs) and secondary organic aerosol (SOA) well before 1750 A.D, possibly causing climate effects through aerosol-radiation and aerosol-cloud interactions. Two numerical emission models LPJ-GUESS and MEGAN were used to quantify the changes in aerosol forming BVOC emissions in the past millennium. A chemical transport model of the atmosphere (GEOS-Chem-TOMAS) was driven with those BVOC emissions to quantify the effects on radiation caused by millennial changes in SOA. We found that global isoprene emissions decreased after 1800 A.D. by about 12% - 15%. This decrease was dominated by losses of natural vegetation, whereas monoterpene and sesquiterpene emissions increased by about 2% - 10%, driven mostly by rising surface air temperatures. From 1000 A.D. to 1800 A.D, isoprene, monoterpene and sesquiterpene emissions decline by 3% - 8% driven by both, natural vegetation losses, and the moderate global cooling between the medieval climate anomaly and the little ice age. The millennial reduction in BVOC emissions lead to a 0.5% to 2% reduction in climatically relevant aerosol particles (> 80 nm) and cause a direct radiative forcing between +0.02 W/m² and +0.07 W/m², and an indirect radiative forcing between -0.02 W/m² and +0.02 W/m².

Remote Sensing of Aerosol and Aerosol Radiative Forcing of Climate from EOS Terra MODIS Instrument

NASA Technical Reports Server (NTRS)

Kaufman, Yoram; Tanre, Didier; Remer, Lorraine; Einaudi, Franco (Technical Monitor)

2000-01-01

The recent launch of EOS-Terra into polar orbit has begun to revolutionize remote sensing of aerosol and their effect on climate. Terra has five instruments, two of them,Moderate Resolution Imaging Spectroradiometer (MODIS) and Multiangle Imaging Spectro-Radiometer (MISR) are designed to monitor global aerosol in two different complementary ways. Here we shall discuss the use of the multispectral measurements of MODIS to derive: (1) the global distribution of aerosol load (and optical thickness) over ocean and land; (2) to measure the impact of aerosol on reflection of sunlight to space; and (3) to measure the ability of aerosol to absorb solar radiation. These measurements have direct applications on the understanding of the effect of aerosol on climate, the ability to predict climate change, and on the monitoring of dust episodes and man-made pollution. Principles of remote sensing of aerosol from MODIS will be discussed and first examples of measurements from MODIS will be provided.

Assessment of Aerosol Optical Property and Radiative Effect for the Layer Decoupling Cases over the Northern South China Sea During the 7-SEAS Dongsha Experiment

NASA Technical Reports Server (NTRS)

Pani, Shantau Kumar; Wang, Sheng-Hsiang; Lin, Neng-Huei; Tsay, Si-Chee; Lolli, Simone; Chuang, Ming-Tung; Lee, Chung-Te; Chantara, Somporn; Yu, Jin-Yi

2016-01-01

The aerosol radiative effect can be modulated by the vertical distribution and optical properties of aerosols, particularly when aerosol layers are decoupled. Direct aerosol radiative effects over the northern South China Sea (SCS) were assessed by incorporating an observed data set of aerosol optical properties obtained from the Seven South East Asian Studies (7-SEAS)/Dongsha Experiment into a radiative transfer model. Aerosol optical properties for a two-layer structure of aerosol transport were estimated. In the radiative transfer calculations, aerosol variability (i.e., diversity of source region, aerosol type, and vertical distribution) for the complex aerosol environment was also carefully quantified. The column-integrated aerosol optical depth (AOD) at 500nm was 0.1-0.3 for near-surface aerosols and increased 1-5 times in presence of upper layer biomass-burning aerosols. A case study showed the strong aerosol absorption (single-scattering albedo (omega) approx. = 0.92 at 440nm wavelength) exhibited by the upper layer when associated with predominantly biomass-burning aerosols, and the omega (approx. = 0.95) of near-surface aerosols was greater than that of the upper layer aerosols because of the presence of mixed type aerosols. The presence of upper level aerosol transport could enhance the radiative efficiency at the surface (i.e., cooling) and lower atmosphere (i.e., heating) by up to -13.7 and +9.6W/sq m2 per AOD, respectively. Such enhancement could potentially modify atmospheric stability, can influence atmospheric circulation, as well as the hydrological cycle over the tropical and low-latitude marginal northern SCS.

Assessment of aerosol optical property and radiative effect for the layer decoupling cases over the northern South China Sea during the 7-SEAS/Dongsha Experiment

NASA Astrophysics Data System (ADS)

Pani, Shantanu Kumar; Wang, Sheng-Hsiang; Lin, Neng-Huei; Tsay, Si-Chee; Lolli, Simone; Chuang, Ming-Tung; Lee, Chung-Te; Chantara, Somporn; Yu, Jin-Yi

2016-05-01

The aerosol radiative effect can be modulated by the vertical distribution and optical properties of aerosols, particularly when aerosol layers are decoupled. Direct aerosol radiative effects over the northern South China Sea (SCS) were assessed by incorporating an observed data set of aerosol optical properties obtained from the Seven South East Asian Studies (7-SEAS)/Dongsha Experiment into a radiative transfer model. Aerosol optical properties for a two-layer structure of aerosol transport were estimated. In the radiative transfer calculations, aerosol variability (i.e., diversity of source region, aerosol type, and vertical distribution) for the complex aerosol environment was also carefully quantified. The column-integrated aerosol optical depth (AOD) at 500 nm was 0.1-0.3 for near-surface aerosols and increased 1-5 times in presence of upper layer biomass-burning aerosols. A case study showed the strong aerosol absorption (single-scattering albedo (ω) ≈ 0.92 at 440 nm wavelength) exhibited by the upper layer when associated with predominantly biomass-burning aerosols, and the ω (≈0.95) of near-surface aerosols was greater than that of the upper layer aerosols because of the presence of mixed type aerosols. The presence of upper level aerosol transport could enhance the radiative efficiency at the surface (i.e., cooling) and lower atmosphere (i.e., heating) by up to -13.7 and +9.6 W m-2 per AOD, respectively. Such enhancement could potentially modify atmospheric stability, can influence atmospheric circulation, as well as the hydrological cycle over the tropical and low-latitude marginal northern SCS.

Combined multispectral/hyperspectral remote sensing of tropospheric aerosols for quantification of their direct radiative effect

NASA Astrophysics Data System (ADS)

McGarragh, Gregory R.

Scattering and absorption of solar radiation by aerosols in the atmosphere has a direct radiative effect on the climate of the Earth. Unfortunately, according to the IPCC the uncertainties in aerosol properties and their effect on the climate system represent one of the largest uncertainties in climate change research. Related to aerosols, one of the largest uncertainties is the fraction of the incident radiation that is scattered rather than absorbed, or their single scattering albedo. In fact, differences in single scattering albedo have a significant impact on the magnitude of the cooling effect of aerosols (opposite to that of greenhouse gasses) which can even have a warming effect for strongly absorbing aerosols. Satellites provide a unique opportunity to measure aerosol properties on a global scale. Traditional approaches use multispectral measurements of intensity at a single view angle to retrieve at most two aerosol parameters over land but it is being realized that more detail is required for accurate quantification of the direct effect of aerosols, in particular its anthropogenic component, and therefore more measurement information is required. One approach to more advanced measurements is to use not only intensity measurements but also polarimetric measurements and to use multiple view angles. In this work we explore another alternative: the use of hyperspectral measurements in molecular absorption bands. Our study can be divided into three stages the first of which is the development of a fast radiative transfer model for rapid simulation of measurements. Our approach is matrix operator based and uses the Pade approximation for the matrix exponential to evaluate the homogeneous solution. It is shown that the method is two to four times faster than the standard and efficient discrete ordinate technique and is accurate to the 6th decimal place. The second part of our study forms the core and is divided into two chapters the first of which is a rigorous

Aerosol Direct Radiative Effect at the Top of the Atmosphere Over Cloud Free Ocean Derived from Four Years of MODIS Data

NASA Technical Reports Server (NTRS)

Remer, L. A.; Kaufman, Y. J.

2006-01-01

A four year record of MODIS spaceborne data provides a new measurement tool to assess the aerosol direct radiative effect at the top of the atmosphere. MODIS derives the aerosol optical thickness and microphysical properties from the scattered sunlight at 0.55-2.1 microns. The monthly MODIS data used here are accumulated measurements across a wide range of view and scattering angles and represent the aerosol s spectrally resolved angular properties. We use these data consistently to compute with estimated accuracy of +/-0.6W/sq m the reflected sunlight by the aerosol over global oceans in cloud free conditions. The MODIS high spatial resolution (0.5 km) allows observation of the aerosol impact between clouds that can be missed by other sensors with larger footprints. We found that over the clear-sky global ocean the aerosol reflected 5.3+/-0.6W/sq m with an average radiative efficiency of 49+/-2W/sq m per unit optical thickness. The seasonal and regional distribution of the aerosol radiative effects are discussed. The analysis adds a new measurement perspective to a climate change problem dominated so far by models.

Trends in surface solar radiation in Spain since the 1980s: the role of the changes in the radiative effects of aerosols and clouds

NASA Astrophysics Data System (ADS)

Sanchez-Lorenzo, Arturo; Mateos, David; Wild, Martin; Calbó, Josep; Antón, Manuel; Enriquez-Alonso, Aaron; Sanchez-Romero, Alex

2014-05-01

There is a growing interest in the study of decadal variations in surface solar radiation, although the analyses of long-term time series in some areas with major gaps in observations, such as in Spain, are still pending. In the first part of this work, a previously published surface solar radiation dataset in Spain is described (for more details, see Sanchez-Lorenzo et al., 2013) based on the longest series with ground-based records of global and diffuse solar radiation, most of them starting in the early 1980s and ending in 2012. Particular emphasis is placed upon the homogenization of this dataset in order to ensure the reliability of the trends. The linear trend in the mean annual series of global solar radiation shows a significant increase since 1981 of 4.0 Wm-2 (or 2.4 %) per decade. These results are in line with the increase of global solar radiation (i.e. brightening period) reported at many worldwide observation sites (Wild, 2009). In addition, the annual mean diffuse solar radiation series shows a significant decrease during the last three decades, but it is disturbed by strong increases in 1983 and 1991-1992, which might reflect the effects of the El Chichón and Pinatubo volcanic eruptions as a result of enhanced scattering of the aerosols emitted during these large volcanic eruptions. As clouds and aerosols are the main sources of uncertainty in the determination of the energy balance of the Earth, there is a growing interest in the evaluation of their radiative effects and their impact on the decadal variability of the surface solar radiation. Hence, in the second part of this work, the changes of the combined radiative effects of clouds and aerosols in Spain since the 1980s are investigated (for more details, see Mateos et al., 2013). In particular, the global solar radiation data above mentioned and radiative transfer simulations fed with reanalysis data of ozone, water vapour and surface albedo, are used to evaluate the cloud and aerosol

A Novel Method for Estimating Shortwave Direct Radiative Effect of Above-Cloud Aerosols Using CALIOP and MODIS Data

NASA Technical Reports Server (NTRS)

Zhang, Z.; Meyer, K.; Platnick, S.; Oreopoulos, L.; Lee, D.; Yu, H.

2014-01-01

This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It accounts for the overlapping of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure. Effects of sub-grid scale cloud and aerosol variations on DRE are accounted for. It is computationally efficient through using grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table in radiative transfer calculations. We verified that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous shortwave DRE that generally agrees with more rigorous pixel-level computation within 4. We have also computed the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global ocean based on 4 yr of CALIOP and MODIS data. We found that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds.

Satellite Estimates of the Direct Radiative Forcing of Biomass Burning Aerosols Over South America and Africa

NASA Technical Reports Server (NTRS)

Christopher, Sundar A.; Wang, Min; Kliche, Donna V.; Berendes, Todd; Welch, Ronald M.; Yang, S.K.

1997-01-01

Atmospheric aerosol particles, both natural and anthropogenic are important to the earth's radiative balance. Therefore it is important to provide adequate validation information on the spatial, temporal and radiative properties of aerosols. This will enable us to predict realistic global estimates of aerosol radiative effects more confidently. The current study utilizes 66 AVHRR LAC (Local Area Coverage) and coincident Earth Radiation Budget Experiment (ERBE) images to characterize the fires, smoke and radiative forcings of biomass burning aerosols over four major ecosystems of South America.

Reallocation in modal aerosol models: impacts on predicting aerosol radiative effects

NASA Astrophysics Data System (ADS)

Korhola, T.; Kokkola, H.; Korhonen, H.; Partanen, A.-I.; Laaksonen, A.; Lehtinen, K. E. J.; Romakkaniemi, S.

2013-08-01

In atmospheric modelling applications the aerosol particle size distribution is commonly represented by modal approach, in which particles in different size ranges are described with log-normal modes within predetermined size ranges. Such method includes numerical reallocation of particles from a mode to another for example during particle growth, leading to potentially artificial changes in the aerosol size distribution. In this study we analysed how this reallocation affects climatologically relevant parameters: cloud droplet number concentration, aerosol-cloud interaction coefficient and light extinction coefficient. We compared these parameters between a modal model with and without reallocation routines, and a high resolution sectional model that was considered as a reference model. We analysed the relative differences of the parameters in different experiments that were designed to cover a wide range of dynamic aerosol processes occurring in the atmosphere. According to our results, limiting the allowed size ranges of the modes and the following numerical remapping of the distribution by reallocation, leads on average to underestimation of cloud droplet number concentration (up to 100%) and overestimation of light extinction (up to 20%). The analysis of aerosol first indirect effect is more complicated as the ACI parameter can be either over- or underestimated by the reallocating model, depending on the conditions. However, for example in the case of atmospheric new particle formation events followed by rapid particle growth, the reallocation can cause around average 10% overestimation of the ACI parameter. Thus it is shown that the reallocation affects the ability of a model to estimate aerosol climate effects accurately, and this should be taken into account when using and developing aerosol models.

CLouds, and Aerosols Radiative Impacts and Forcing: Year 2016 (CLARIFY-2016)

NASA Astrophysics Data System (ADS)

Haywood, J. M.; Bellouin, N.; Carslaw, K. S.; Coe, H.; Field, P.; Highwood, E. J.; Redemann, J.; Stier, P.; Wood, R.; Zuidema, P.

2013-12-01

Strongly absorbing biomass burning aerosols (BBAs) exist above highly reflectant stratocumulus clouds in the SE Atlantic with implications on the direct (e.g. Haywood et al., 2003), semi-direct (e.g. Johnson et al., 2006), and indirect effect of aerosols, implications on the remote sensing of cloud optical properties, development of clouds and feedback processes. Here, we present an analysis of modelled estimates of the direct effect using twelve models from the AEROCOM project (Myhre et al., 2013) to show that estimates of the direct effect in SE Atlantic range from strongly negative to strongly positive. Furthermore, we evaluate the performance of the HadGEM2 model and show it cannot replicate the extreme values of positive forcing inferred from high spectral resolution satellite retrievals. By examining patterns of deposition, we infer that the indirect effect from biomass burning aerosols is very limited in the model, but without detailed measurements we are unsure of the validity of this inference. We conclude that the SE Atlantic is therefore of key importance in determining the radiative forcing of biomass burning aerosols and provides a very stringent test for global climate models as they need to accurately represent the geographic distribution of the aerosol optical depth, the wavelength dependent aerosol single scattering albedo, the vertical profile of the aerosol, the geographic distribution of the cloud, the cloud fraction, the cloud liquid water content, the cloud droplet effective radii, and the vertical profile of the cloud. These results are used as scientific rationale to justify a new measurement campaign: CLouds and Aerosol Radiative Impacts and Forcing: Year-2016 (CLARIFY-2016). Haywood, J.M., Osborne, S.R. Francis, P.N., Keil, A., Formenti, P., Andreae, M.O., and Kaye, P.H., The mean physical and optical properties of regional haze dominated by biomass burning aerosol measured from the C-130 aircraft during SAFARI 2000, J. Geophys. Res., 108

A comparison of uncertainties in the aerosol direct radiative effect in the SE U.S. calculated using satellite-based and ground-based aerosol properties

NASA Astrophysics Data System (ADS)

Sherman, J. P.

2017-12-01

Satellite-retrieved aerosol optical depth is typically used for measurement-based estimates of the aerosol direct radiative effect (DRE) on solar radiation, on both global and regional scales. The SE U.S. is one of only a few regions not to have warmed during the 20th century and is home to some of the highest summertime levels of biogenic and sulfate aerosols in the U.S. While decreases in aerosol optical depth over the past few decades have likely reduced the cooling effect of aerosols in the region, satellite-derived estimates of aerosol DRE alone may not be sufficient to study long-term DRE trends and the roles played by changing AOD and aerosol optical properties. Appalachian State University (APP) in Boone, NC is home to the only co-located NASA AERONET, NOAA ESRL, and (active) NASA MPLNET sites in the U.S. and is well-positioned to validate satellite-based aerosol retrievals and better constrain background aerosol DRE in regional climate models. As part of the first multi-year `ground truth' DRE study in the SE U.S., Sherman and McComiskey (2017) applied nearly four years of spectral AOD from the APP AERONET site, along with single-scattering albedo(SSA) and asymmetry parameter from the APP NOAA ESRL site, as inputs to the SBDART Radiative Transfer model to calculate seasonal dependence of aerosol DRE and DRE uncertainties at the top-of-atmosphere and at the surface. Clear sky aerosol DRE uncertainty at the TOA (surface) above APP ranges from 0.44 Wm-2 (0.73 Wm-2) for DEC to 0.90 Wm-2 (1.3 Wm-2) for JUN. Expressed as a fraction of seasonal-mean DRE, these uncertainties are 12-20% for all seasons except winter, when they are close to 50%. Use of MODIS or MISR AOD in place of AERONET increases these uncertainties by factors of 2.5 to 5 and DRE uncertainties are dominated by AOD uncertainty for all seasons. The use of SSA from OMI or MISR further increases the DRE uncertainties, especially during the higher AOD summer months, when DRE sensitivity to aerosol

Impact of varying lidar measurement and data processing techniques in evaluating cirrus cloud and aerosol direct radiative effects

NASA Astrophysics Data System (ADS)

Lolli, Simone; Madonna, Fabio; Rosoldi, Marco; Campbell, James R.; Welton, Ellsworth J.; Lewis, Jasper R.; Gu, Yu; Pappalardo, Gelsomina

2018-03-01

In the past 2 decades, ground-based lidar networks have drastically increased in scope and relevance, thanks primarily to the advent of lidar observations from space and their need for validation. Lidar observations of aerosol and cloud geometrical, optical and microphysical atmospheric properties are subsequently used to evaluate their direct radiative effects on climate. However, the retrievals are strongly dependent on the lidar instrument measurement technique and subsequent data processing methodologies. In this paper, we evaluate the discrepancies between the use of Raman and elastic lidar measurement techniques and corresponding data processing methods for two aerosol layers in the free troposphere and for two cirrus clouds with different optical depths. Results show that the different lidar techniques are responsible for discrepancies in the model-derived direct radiative effects for biomass burning (0.05 W m-2 at surface and 0.007 W m-2 at top of the atmosphere) and dust aerosol layers (0.7 W m-2 at surface and 0.85 W m-2 at top of the atmosphere). Data processing is further responsible for discrepancies in both thin (0.55 W m-2 at surface and 2.7 W m-2 at top of the atmosphere) and opaque (7.7 W m-2 at surface and 11.8 W m-2 at top of the atmosphere) cirrus clouds. Direct radiative effect discrepancies can be attributed to the larger variability of the lidar ratio for aerosols (20-150 sr) than for clouds (20-35 sr). For this reason, the influence of the applied lidar technique plays a more fundamental role in aerosol monitoring because the lidar ratio must be retrieved with relatively high accuracy. In contrast, for cirrus clouds, with the lidar ratio being much less variable, the data processing is critical because smoothing it modifies the aerosol and cloud vertically resolved extinction profile that is used as input to compute direct radiative effect calculations.

Stratospheric Aerosols for Solar Radiation Management

NASA Astrophysics Data System (ADS)

Kravitz, Ben

SRM in the context of this entry involves placing a large amount of aerosols in the stratosphere to reduce the amount of solar radiation reaching the surface, thereby cooling the surface and counteracting some of the warming from anthropogenic greenhouse gases. The way this is accomplished depends on the specific aerosol used, but the basic mechanism involves backscattering and absorbing certain amounts of solar radiation aloft. Since warming from greenhouse gases is due to longwave (thermal) emission, compensating for this warming by reduction of shortwave (solar) energy is inherently imperfect, meaning SRM will have climate effects that are different from the effects of climate change. This will likely manifest in the form of regional inequalities, in that, similarly to climate change, some regions will benefit from SRM, while some will be adversely affected, viewed both in the context of present climate and a climate with high CO2 concentrations. These effects are highly dependent upon the means of SRM, including the type of aerosol to be used, the particle size and other microphysical concerns, and the methods by which the aerosol is placed in the stratosphere. SRM has never been performed, nor has deployment been tested, so the research up to this point has serious gaps. The amount of aerosols required is large enough that SRM would require a major engineering endeavor, although SRM is potentially cheap enough that it could be conducted unilaterally. Methods of governance must be in place before deployment is attempted, should deployment even be desired. Research in public policy, ethics, and economics, as well as many other disciplines, will be essential to the decision-making process. SRM is only a palliative treatment for climate change, and it is best viewed as part of a portfolio of responses, including mitigation, adaptation, and possibly CDR. At most, SRM is insurance against dangerous consequences that are directly due to increased surface air

Satellite-derived aerosol radiative forcing from the 2004 British Columbia wildfires

USGS Publications Warehouse

Guo, Song; Leighton, H.

2008-01-01

The British Columbia wildfires of 2004 was one of the largest wildfire events in the last ten years in Canada. Both the shortwave and longwave smoke aerosol radiative forcing at the top-of-atmosphere (TOA) are investigated using data from the Moderate Resolution Imaging Spectroradiometer (MODIS) and the Clouds and the Earth's Radiant Energy System (CERES) instruments. Relationships between the radiative forcing fluxes (??F) and wildfire aerosol optical thickness (AOT) at 0.55 ??m (??0.55) are deduced for both noontime instantaneous forcing and diurnally averaged forcing. The noontime averaged instantaneous shortwave and longwave smoke aerosol radiative forcing at the TOA are 45.8??27.5 W m-2 and -12.6??6.9 W m-2, respectively for a selected study area between 62??N and 68??N in latitude and 125??W and 145??W in longitude over three mainly clear-sky days (23-25 June). The derived diurnally averaged smoke aerosol shortwave radiative forcing is 19.9??12.1 W m-2 for a mean ??0.55 of 1.88??0.71 over the same time period. The derived ??F-?? relationship can be implemented in the radiation scheme used in regional climate models to assess the effect of wildfire aerosols.

Variability of aerosol optical depth and aerosol radiative forcing over Northwest Himalayan region

NASA Astrophysics Data System (ADS)

Saheb, Shaik Darga; Kant, Yogesh; Mitra, D.

2016-05-01

In recent years, the aerosol loading in India is increasing that has significant impact on the weather/climatic conditions. The present study discusses the analysis of temporal (monthly and seasonal) variation of aerosol optical depth(AOD) by the ground based observations from sun photometer and estimate the aerosol radiative forcing and heating rate over selected station Dehradun in North western Himalayas, India during 2015. The in-situ measurements data illustrate that the maximum seasonal average AOD observed during summer season AOD at 500nm ≍ 0.59+/-0.27 with an average angstrom exponent, α ≍0.86 while minimum during winter season AOD at 500nm ≍ 0.33+/-0.10 with angstrom exponent, α ≍1.18. The MODIS and MISR derived AOD was also compared with the ground measured values and are good to be in good agreement. Analysis of air mass back trajectories using HYSPLIT model reveal that the transportation of desert dust during summer months. The Optical Properties of Aerosols and clouds (OPAC) model was used to compute the aerosol optical properties like single scattering albedo (SSA), Angstrom coefficient (α) and Asymmetry(g) parameter for each day of measurement and they are incorporated in a Discrete Ordinate Radiative Transfer model, i.e Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) to estimate the direct short-wave (0.25 to 4 μm) Aerosol Radiative forcing at the Surface (SUR), the top-of-atmosphere (TOA) and Atmosphere (ATM). The maximum Aerosol Radiative Forcing (ARF) was observed during summer months at SUR ≍ -56.42 w/m2, at TOA ≍-21.62 w/m2 whereas in ATM ≍+34.79 w/m2 with corresponding to heating rate 1.24°C/day with in lower atmosphere.

Significance of aerosol radiative effect in energy balance control on global precipitation change

DOE Office of Scientific and Technical Information (OSTI.GOV)

Suzuki, Kentaroh; Stephens, Graeme L.; Golaz, Jean-Christophe

Historical changes of global precipitation in the 20th century simulated by a climate model are investigated. The results simulated with alternate configurations of cloud microphysics are analyzed in the context of energy balance controls on global precipitation, where the latent heat changes associated with the precipitation change is nearly balanced with changes to atmospheric radiative cooling. The atmospheric radiative cooling is dominated by its clear-sky component, which is found to correlate with changes to both column water vapor and aerosol optical depth (AOD). The water vapor-dependent component of the clear-sky radiative cooling is then found to scale with global temperaturemore » change through the Clausius–Clapeyron relationship. This component results in a tendency of global precipitation increase with increasing temperature at a rate of approximately 2%K -1. Another component of the clear-sky radiative cooling, which is well correlated with changes to AOD, is also found to vary in magnitude among different scenarios with alternate configurations of cloud microphysics that controls the precipitation efficiency, a major factor influencing the aerosol scavenging process that can lead to different aerosol loadings. These results propose how different characteristics of cloud microphysics can cause different aerosol loadings that in turn perturb global energy balance to significantly change global precipitation. This implies a possible coupling of aerosol–cloud interaction with aerosol–radiation interaction in the context of global energy balance.« less

Significance of aerosol radiative effect in energy balance control on global precipitation change

DOE PAGES

Suzuki, Kentaroh; Stephens, Graeme L.; Golaz, Jean-Christophe

2017-10-17

Historical changes of global precipitation in the 20th century simulated by a climate model are investigated. The results simulated with alternate configurations of cloud microphysics are analyzed in the context of energy balance controls on global precipitation, where the latent heat changes associated with the precipitation change is nearly balanced with changes to atmospheric radiative cooling. The atmospheric radiative cooling is dominated by its clear-sky component, which is found to correlate with changes to both column water vapor and aerosol optical depth (AOD). The water vapor-dependent component of the clear-sky radiative cooling is then found to scale with global temperaturemore » change through the Clausius–Clapeyron relationship. This component results in a tendency of global precipitation increase with increasing temperature at a rate of approximately 2%K -1. Another component of the clear-sky radiative cooling, which is well correlated with changes to AOD, is also found to vary in magnitude among different scenarios with alternate configurations of cloud microphysics that controls the precipitation efficiency, a major factor influencing the aerosol scavenging process that can lead to different aerosol loadings. These results propose how different characteristics of cloud microphysics can cause different aerosol loadings that in turn perturb global energy balance to significantly change global precipitation. This implies a possible coupling of aerosol–cloud interaction with aerosol–radiation interaction in the context of global energy balance.« less

Impacts of Aerosol Direct Effects on the South Asian Climate: Assessment of Radiative Feedback Processes Using Model Simulations and Satellite/Surface Measurements

NASA Technical Reports Server (NTRS)

Wang, Sheng-Hsiang; Gautam, Ritesh; Lau, William K. M.; Tsay, Si-Chee; Sun, Wen-Yih; Kim, Kyu-Myong; Chern, Jiun-Dar; Hsu, Christina; Lin, Neng-Huei

2011-01-01

Current assessment of aerosol radiative effect is hindered by our incomplete knowledge of aerosol optical properties, especially absorption, and our current inability to quantify physical and microphysical processes. In this research, we investigate direct aerosol radiative effect over heavy aerosol loading areas (e.g., Indo-Gangetic Plains, South/East Asia) and its feedbacks on the South Asian climate during the pre-monsoon season (March-June) using the Purdue Regional Climate Model (PRCM) with prescribed aerosol data derived by the NASA Goddard Earth Observing System Model (GEOS-5). Our modeling domain covers South and East Asia (60-140E and 0-50N) with spatial resolutions of 45 km in horizontal and 28 layers in vertical. The model is integrated from 15 February to 30 June 2008 continuously without nudging (i.e., only forced by initial/boundary conditions). Two numerical experiments are conducted with and without the aerosol-radiation effects. Both simulations are successful in reproducing the synoptic patterns on seasonal-to-interannual time scales and capturing a pre-monsoon feature of the northward rainfall propagation over Indian region in early June which shown in Tropical Rainfall Measuring Mission (TRMM) observation. Preliminary result suggests aerosol-radiation interactions mainly alter surface-atmosphere energetics and further result in an adjustment of the vertical temperature distribution in lower atmosphere (below 700 hPa). The modifications of temperature and associated rainfall and circulation feedbacks on the regional climate will be discussed in the presentation.

High-power laser radiation in atmospheric aerosols: Nonlinear optics of aerodispersed media

NASA Astrophysics Data System (ADS)

Zuev, V. E.; Zemlianov, A. A.; Kopytin, Iu. D.; Kuzikovskii, A. V.

The bulk of this book contains the results of investigations carried out at the Institute of Atmospheric Optics, Siberian Branch, USSR Academy of Science with the participation of the authors. The microphysical and optical characteristics of atmospheric aerosols are considered, taking into account light scattering by a single aerosol particle, light scattering by a system of particles, the scattering phase matrix, light scattering by clouds and fogs, light scattering by hazes, and scattering phase functions of polydispersed aerosols. Other topics studies are related to low-energy (subexplosive) effects of radiation on individual particles, the formation of clear zones in clouds and fogs due to the vaporization of droplets under regular regimes, self-action of a wave beam in a water aerosol under conditions of regular droplet vaporization, laser beam propagation through an explosively evaporating water-droplet aerosol, the propagation of high-power laser radiation through hazes, the ionization and optical breakdown in aerosol media, and laser monitoring of a turbid atmosphere using nonlinear effects.

Radiative forcing of the desert aerosol at Ouarzazate (Morocco)

NASA Astrophysics Data System (ADS)

Tahiri, Abdelouahid; Diouri, Mohamed

2018-05-01

The atmospheric aerosol contributes to the definition of the climate with direct effect, the diffusion and absorption of solar and terrestrial radiations, and indirect, the cloud formation process where aerosols behave as condensation nuclei and alter the optical properties. Satellites and ground-based networks (solar photometers) allow the terrestrial aerosol observation and the determination of impact. Desert aerosol considered among the main types of tropospheric aerosols whose optical property uncertainties are still quite important. The analysis concerns the optical parameters recorded in 2015 at Ouarzazate solar photometric station (AERONET/PHOTONS network, http://aeronet.gsfc.nasa.gov/) close to Saharan zone. The daily average aerosol optical depthτaer at 0.5μm, are relatively high in summer and less degree in spring (from 0.01 to 1.82). Daily average of the Angstrom coefficients α vary between 0.01 and 1.55. The daily average of aerosol radiative forcing at the surface range between -150W/m2 and -10 W/m2 with peaks recorded in summer, characterized locally by large loads of desert aerosol in agreement with the advections of the Southeast of Morocco. Those recorded at the Top of the atmosphere show a variation from -74 W/m2 to +24 W/m2

Aerosols and their influence on radiation partitioning and savanna productivity in northern Australia

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kanniah, K. D.; Beringer, J.; Tapper, N. J.

2010-05-01

We investigated the effect of aerosols and clouds on the Net Ecosystem Productivity (NEP) of savannas in northern Australia using aerosol optical depth, clouds and radiation data from the Atmospheric Radiation Measurement (ARM) site in Darwin and carbon flux data measured from eddy covariance techniques from a site at Howard Springs, 35km southeast of Darwin. Generally we found that the concentration of aerosols in this region was relatively low than observed at other sites, therefore the proportion of diffuse radiation reaching the earths surface was only ~ 30%. As a result, we observed only a modest change in carbon uptakemore » under aerosol laden skies and there was no significant difference for dry season Radiation Use Efficiency (RUE) between clear sky, aerosols or thin clouds. On the other hand thick clouds in the wet season produce much more diffuse radiation than aerosols or thin clouds and therefore the initial canopy quantum efficiency was seen to increase 45 and 2.5 times more than under thin clouds and aerosols respectively. The normalized carbon uptake under thick clouds is 57% and 50% higher than under aerosols and thin clouds respectively even though the total irradiance received under thick clouds was reduced 59% and 50% than under aerosols and thin clouds respectively. However, reduction in total irradiance decreases the mean absolute carbon uptake as much as 22% under heavy cloud cover compared to thin clouds or aerosols. Thus, any increase in aerosol concentration or cloud cover that can enhance the diffuse component may have large impacts on productivity in this region.« less

Radiative effects of absorbing aerosols over northeastern India: Observations and model simulations

NASA Astrophysics Data System (ADS)

Gogoi, Mukunda M.; Babu, S. Suresh; Moorthy, K. Krishna; Bhuyan, Pradip Kumar; Pathak, Binita; Subba, Tamanna; Chutia, Lakhima; Kundu, Shyam Sundar; Bharali, Chandrakala; Borgohain, Arup; Guha, Anirban; De, Barin Kumar; Singh, Brajamani; Chin, Mian

2017-01-01

Multiyear measurements of spectral properties of aerosol absorption are examined over four geographically distinct locations of northeastern India. Results indicated significant spatiotemporal variation in aerosol absorption coefficients (σabs) with highest values in winter and lowest in monsoon. The western parts of the region, close to the outflow of Indo-Gangetic Plains, showed higher values of σabs and black carbon (BC) concentration—mostly associated with fossil fuel combustion. But, the eastern parts showed higher contributions from biomass-burning aerosols, as much as 20-25% to the total aerosol absorption, conspicuously during premonsoon season. This is attributed to a large number of burning activities over the Southeast Asian region, as depicted from Moderate Resolution Imaging Spectroradiometer fire count maps, whose spatial extent and magnitude peaks during March/April. The nearly consistent high values of aerosol index (AI) and layer height from Ozone Monitoring Instrument indicate the presence of absorbing aerosols in the upper atmosphere. The observed seasonality has been captured fairly well by Goddard Chemistry Aerosol Radiation and Transport (GOCART) as well as Weather Research and Forecasting-Chemistry (WRF-Chem) model simulations. The ratio of column-integrated optical depths due to particulate organic matter and BC from GOCART showed good coincidence with satellite-based observations, indicating the increased vertical dispersion of absorbing aerosols, probably by the additional local convection due to higher fire radiative power caused by the intense biomass-burning activities. In the WRF-Chem though underperformed by different magnitude in winter, the values are closer or overestimated near the burnt areas. Atmospheric forcing due to BC was highest ( 30 Wm-2) over the western part associated with the fossil fuel combustion.

Direct Aerosol Radiative Forcing Based on Combined A-Train Observations: Towards All-sky Estimates and Attribution to Aerosol Type

NASA Technical Reports Server (NTRS)

Redemann, Jens; Shinozuka, Y.; Kacenelenbogen, M.; Russell, P.; Vaughan, M.; Ferrare, R.; Hostetler, C.; Rogers, R.; Burton, S.; Livingston, J.;

Simulating Changes in Tropospheric Aerosol Burden and its Radiative Effects across the Northern Hemisphere: Contrasting Multi-Decadal Trends between Asia and North America

EPA Science Inventory

Though aerosol radiative effects have been recognized as some of the largest sources of uncertainty among the forcers of climate change, the verification of the spatial and temporal variability of the magnitude and directionality of aerosol radiative forcing has remained challeng...

Impact of springtime biomass-burning aerosols on radiative forcing over northern Thailand during the 7SEAS campaign

NASA Astrophysics Data System (ADS)

Pani, Shantanu Kumar; Wang, Sheng-Hsiang; Lin, Neng-Huei; Lee, Chung-Te; Tsay, Si-Chee; Holben, Brent; Janjai, Serm; Hsiao, Ta-Chih; Chuang, Ming-Tung; Chantara, Somporn

2016-04-01

Biomass-burning (BB) aerosols are the significant contributor to the regional/global aerosol loading and radiation budgets. BB aerosols affect the radiation budget of the earth and atmosphere by scattering and absorbing directly the incoming solar and outgoing terrestrial radiation. These aerosols can exert either cooling or warming effect on climate, depending on the balance between scattering and absorption. BB activities in the form of wildland forest fires and agricultural crop burning are very pronounced in the Indochina peninsular regions in Southeast Asia mainly in spring (late February to April) season. The region of interest includes Doi Ang Khang (19.93° N, 99.05° E, 1536 msl) in northern Thailand, as part of the Seven South East Asian Studies (7-SEAS)/BASELInE (Biomass-burning Aerosols & Stratocumulus Environment: Lifecycles & Interactions Experiment) campaign in 2013. In this study, for the first time, the direct aerosol radiative effects of BB aerosols over near-source BB emissions, during the peak loading spring season, in northern Indochina were investigated by using ground-based physical, chemical, and optical properties of aerosols as well as the aerosol optical and radiative transfer models. Information on aerosol parameters in the field campaign was used in the OPAC (Optical Properties of Aerosols and Clouds) model to estimate various optical properties corresponding to aerosol compositions. Clear-sky shortwave direct aerosol radiative effects were further estimated with a raditive transfer model SBDART (Santa Barbara DISORT Atmospheric Radiative Transfer). The columnar aerosol optical depth (AOD500) was found to be ranged from 0.26 to 1.13 (with the mean value 0.71 ± 0.24). Fine-mode (fine mode fraction ≈0.98, angstrom exponent ≈1.8) and significantly absorbing aerosols (columnar single-scattering albedo ≈0.89, asymmetry-parameter ≈0.67 at 441 nm wavelength) dominated in this region. Water soluble and black carbon (BC) aerosols mainly

Reduced anthropogenic aerosol radiative forcing caused by biogenic new particle formation

NASA Astrophysics Data System (ADS)

Gordon, Hamish; Sengupta, Kamalika; Rap, Alexandru; Duplissy, Jonathan; Frege, Carla; Williamson, Christina; Heinritzi, Martin; Simon, Mario; Yan, Chao; Almeida, João; Tröstl, Jasmin; Nieminen, Tuomo; Ortega, Ismael K.; Wagner, Robert; Dunne, Eimear M.; Adamov, Alexey; Amorim, Antonio; Bernhammer, Anne-Kathrin; Bianchi, Federico; Breitenlechner, Martin; Brilke, Sophia; Chen, Xuemeng; Craven, Jill S.; Dias, Antonio; Ehrhart, Sebastian; Fischer, Lukas; Flagan, Richard C.; Franchin, Alessandro; Fuchs, Claudia; Guida, Roberto; Hakala, Jani; Hoyle, Christopher R.; Jokinen, Tuija; Junninen, Heikki; Kangasluoma, Juha; Kim, Jaeseok; Kirkby, Jasper; Krapf, Manuel; Kürten, Andreas; Laaksonen, Ari; Lehtipalo, Katrianne; Makhmutov, Vladimir; Mathot, Serge; Molteni, Ugo; Monks, Sarah A.; Onnela, Antti; Peräkylä, Otso; Piel, Felix; Petäjä, Tuukka; Praplan, Arnaud P.; Pringle, Kirsty J.; Richards, Nigel A. D.; Rissanen, Matti P.; Rondo, Linda; Sarnela, Nina; Schobesberger, Siegfried; Scott, Catherine E.; Seinfeld, John H.; Sharma, Sangeeta; Sipilä, Mikko; Steiner, Gerhard; Stozhkov, Yuri; Stratmann, Frank; Tomé, Antonio; Virtanen, Annele; Vogel, Alexander Lucas; Wagner, Andrea C.; Wagner, Paul E.; Weingartner, Ernest; Wimmer, Daniela; Winkler, Paul M.; Ye, Penglin; Zhang, Xuan; Hansel, Armin; Dommen, Josef; Donahue, Neil M.; Worsnop, Douglas R.; Baltensperger, Urs; Kulmala, Markku; Curtius, Joachim; Carslaw, Kenneth S.

2016-10-01

The magnitude of aerosol radiative forcing caused by anthropogenic emissions depends on the baseline state of the atmosphere under pristine preindustrial conditions. Measurements show that particle formation in atmospheric conditions can occur solely from biogenic vapors. Here, we evaluate the potential effect of this source of particles on preindustrial cloud condensation nuclei (CCN) concentrations and aerosol-cloud radiative forcing over the industrial period. Model simulations show that the pure biogenic particle formation mechanism has a much larger relative effect on CCN concentrations in the preindustrial atmosphere than in the present atmosphere because of the lower aerosol concentrations. Consequently, preindustrial cloud albedo is increased more than under present day conditions, and therefore the cooling forcing of anthropogenic aerosols is reduced. The mechanism increases CCN concentrations by 20-100% over a large fraction of the preindustrial lower atmosphere, and the magnitude of annual global mean radiative forcing caused by changes of cloud albedo since 1750 is reduced by 0.22 W m-2 (27%) to -0.60 W m-2. Model uncertainties, relatively slow formation rates, and limited available ambient measurements make it difficult to establish the significance of a mechanism that has its dominant effect under preindustrial conditions. Our simulations predict more particle formation in the Amazon than is observed. However, the first observation of pure organic nucleation has now been reported for the free troposphere. Given the potentially significant effect on anthropogenic forcing, effort should be made to better understand such naturally driven aerosol processes.

GCM Simulations of the Aerosol Indirect Effect: Sensitivity to Cloud Parameterization and Aerosol Burden

NASA Technical Reports Server (NTRS)

Menon, Surabi; DelGenio, Anthony D.; Koch, Dorothy; Tselioudis, George; Hansen, James E. (Technical Monitor)

2001-01-01

We describe the coupling of the Goddard Institute for Space Studies (GISS) general circulation model (GCM) to an online sulfur chemistry model and source models for organic matter and sea-salt that is used to estimate the aerosol indirect effect. The cloud droplet number concentration is diagnosed empirically from field experiment datasets over land and ocean that observe droplet number and all three aerosol types simultaneously; corrections are made for implied variations in cloud turbulence levels. The resulting cloud droplet number is used to calculate variations in droplet effective radius, which in turn allows us to predict aerosol effects on cloud optical thickness and microphysical process rates. We calculate the aerosol indirect effect by differencing the top-of-the-atmosphere net cloud radiative forcing for simulations with present-day vs. pre-industrial emissions. Both the first (radiative) and second (microphysical) indirect effects are explored. We test the sensitivity of our results to cloud parameterization assumptions that control the vertical distribution of cloud occurrence, the autoconversion rate, and the aerosol scavenging rate, each of which feeds back significantly on the model aerosol burden. The global mean aerosol indirect effect for all three aerosol types ranges from -1.55 to -4.36 W m(exp -2) in our simulations. The results are quite sensitive to the pre-industrial background aerosol burden, with low pre-industrial burdens giving strong indirect effects, and to a lesser extent to the anthropogenic aerosol burden, with large burdens giving somewhat larger indirect effects. Because of this dependence on the background aerosol, model diagnostics such as albedo-particle size correlations and column cloud susceptibility, for which satellite validation products are available, are not good predictors of the resulting indirect effect.

GCM Simulations of the Aerosol Indirect Effect: Sensitivity to Cloud Parameterization and Aerosol Burden

NASA Technical Reports Server (NTRS)

Menon, Surabi; DelGenio, Anthony D.; Koch, Dorothy; Tselioudis, George; Hansen, James E. (Technical Monitor)

2001-01-01

We describe the coupling of the Goddard Institute for Space Studies (GISS) general circulation model (GCM) to an online sulfur chemistry model and source models for organic matter and sea-salt that is used to estimate the aerosol indirect effect. The cloud droplet number concentration is diagnosed empirically from field experiment datasets over land and ocean that observe droplet number and all three aerosol types simultaneously; corrections are made for implied variations in cloud turbulence levels. The resulting cloud droplet number is used to calculate variations in droplet effective radius, which in turn allows us to predict aerosol effects on cloud optical thickness and microphysical process rates. We calculate the aerosol indirect effect by differencing the top-of-the-atmosphere net cloud radiative forcing for simulations with present-day vs. pre-industrial emissions. Both the first (radiative) and second (microphysical) indirect effects are explored. We test the sensitivity of our results to cloud parameterization assumptions that control the vertical distribution of cloud occurrence, the autoconversion rate, and the aerosol scavenging rate, each of which feeds back significantly on the model aerosol burden. The global mean aerosol indirect effect for all three aerosol types ranges from -1.55 to -4.36 W/sq m in our simulations. The results are quite sensitive to the pre-industrial background aerosol burden, with low pre-industrial burdens giving strong indirect effects, and to a lesser extent to the anthropogenic aerosol burden, with large burdens giving somewhat larger indirect effects. Because of this dependence on the background aerosol, model diagnostics such as albedo-particle size correlations and column cloud susceptibility, for which satellite validation products are available, are not good predictors of the resulting indirect effect.

Intercomparison of shortwave radiative transfer schemes in global aerosol modeling: results from the AeroCom Radiative Transfer Experiment

NASA Astrophysics Data System (ADS)

Randles, C. A.; Kinne, S.; Myhre, G.; Schulz, M.; Stier, P.; Fischer, J.; Doppler, L.; Highwood, E.; Ryder, C.; Harris, B.; Huttunen, J.; Ma, Y.; Pinker, R. T.; Mayer, B.; Neubauer, D.; Hitzenberger, R.; Oreopoulos, L.; Lee, D.; Pitari, G.; Di Genova, G.; Quaas, J.; Rose, Fred G.; Kato, S.; Rumbold, S. T.; Vardavas, I.; Hatzianastassiou, N.; Matsoukas, C.; Yu, H.; Zhang, F.; Zhang, H.; Lu, P.

2012-12-01

In this study we examine the performance of 31 global model radiative transfer schemes in cloud-free conditions with prescribed gaseous absorbers and no aerosols (Rayleigh atmosphere), with prescribed scattering-only aerosols, and with more absorbing aerosols. Results are compared to benchmark results from high-resolution, multi-angular line-by-line radiation models. For purely scattering aerosols, model bias relative to the line-by-line models in the top-of-the atmosphere aerosol radiative forcing ranges from roughly -10 to 20%, with over- and underestimates of radiative cooling at higher and lower sun elevation, respectively. Inter-model diversity (relative standard deviation) increases from ~10 to 15% as sun elevation increases. Inter-model diversity in atmospheric and surface forcing decreases with increased aerosol absorption, indicating that the treatment of multiple-scattering is more variable than aerosol absorption in the models considered. Aerosol radiative forcing results from multi-stream models are generally in better agreement with the line-by-line results than the simpler two-stream schemes. Considering radiative fluxes, model performance is generally the same or slightly better than results from previous radiation scheme intercomparisons. However, the inter-model diversity in aerosol radiative forcing remains large, primarily as a result of the treatment of multiple-scattering. Results indicate that global models that estimate aerosol radiative forcing with two-stream radiation schemes may be subject to persistent biases introduced by these schemes, particularly for regional aerosol forcing.

Intercomparison of shortwave radiative transfer schemes in global aerosol modeling: results from the AeroCom Radiative Transfer Experiment

NASA Astrophysics Data System (ADS)

Randles, C. A.; Kinne, S.; Myhre, G.; Schulz, M.; Stier, P.; Fischer, J.; Doppler, L.; Highwood, E.; Ryder, C.; Harris, B.; Huttunen, J.; Ma, Y.; Pinker, R. T.; Mayer, B.; Neubauer, D.; Hitzenberger, R.; Oreopoulos, L.; Lee, D.; Pitari, G.; Di Genova, G.; Quaas, J.; Rose, F. G.; Kato, S.; Rumbold, S. T.; Vardavas, I.; Hatzianastassiou, N.; Matsoukas, C.; Yu, H.; Zhang, F.; Zhang, H.; Lu, P.

2013-03-01

In this study we examine the performance of 31 global model radiative transfer schemes in cloud-free conditions with prescribed gaseous absorbers and no aerosols (Rayleigh atmosphere), with prescribed scattering-only aerosols, and with more absorbing aerosols. Results are compared to benchmark results from high-resolution, multi-angular line-by-line radiation models. For purely scattering aerosols, model bias relative to the line-by-line models in the top-of-the atmosphere aerosol radiative forcing ranges from roughly -10 to 20%, with over- and underestimates of radiative cooling at lower and higher solar zenith angle, respectively. Inter-model diversity (relative standard deviation) increases from ~10 to 15% as solar zenith angle decreases. Inter-model diversity in atmospheric and surface forcing decreases with increased aerosol absorption, indicating that the treatment of multiple-scattering is more variable than aerosol absorption in the models considered. Aerosol radiative forcing results from multi-stream models are generally in better agreement with the line-by-line results than the simpler two-stream schemes. Considering radiative fluxes, model performance is generally the same or slightly better than results from previous radiation scheme intercomparisons. However, the inter-model diversity in aerosol radiative forcing remains large, primarily as a result of the treatment of multiple-scattering. Results indicate that global models that estimate aerosol radiative forcing with two-stream radiation schemes may be subject to persistent biases introduced by these schemes, particularly for regional aerosol forcing.

Aerosol Direct Radiative Effects Over the Northwest Atlantic, Northwest Pacific, and North Indian Oceans: Estimates Based on In-situ Chemical and Optical Measurements and Chemical Transport Modeling

NASA Astrophysics Data System (ADS)

Bates, T. S.; Anderson, T. L.; Baynard, T.; Bond, T.; Boucher, O.; Carmichael, G.; Clarke, A.; Erlick, C.; Guo, H.; Horowitz, L.; Howell, S.; Kulkarni, S.; Maring, H.; McComiskey, A.; Middlebrook, A.; Noone, K.; O'Dowd, C. D.; Ogren, J. A.; Penner, J.; Quinn, P. K.; Ravishankara, A. R.; Savoie, D. L.; Schwartz, S. E.; Shinozuka, Y.; Tang, Y.; Weber, R. J.; Wu, Y.

2005-12-01

The largest uncertainty in the radiative forcing of climate change over the industrial era is that due to aerosols, a substantial fraction of which is the uncertainty associated with scattering and absorption of shortwave (solar) radiation by anthropogenic aerosols in cloud-free conditions. Quantifying and reducing the uncertainty in aerosol influences on climate is critical to understanding climate change over the industrial period and to improving predictions of future climate change for assumed emission scenarios. Measurements of aerosol properties during major field campaigns in several regions of the globe during the past decade are contributing to an enhanced understanding of atmospheric aerosols and their effects on light scattering and climate. The present study, which focuses on three regions downwind of major urban/population centers (North Indian Ocean during INDOEX, the Northwest Pacific Ocean during ACE-Asia, and the Northwest Atlantic Ocean during ICARTT), incorporates understanding gained from field observations of aerosol distributions and properties into calculations of perturbations in radiative fluxes due to these aerosols. This study evaluates the current state of observations and of two chemical transport models (STEM and MOZART). Measurements of burdens, extinction optical depth, and direct radiative effect of aerosols (change in radiative flux due to total aerosols) are used as measurement-model check points to assess uncertainties. In-situ measured and remotely sensed aerosol properties for each region (mixing state, mass scattering efficiency, single scattering albedo, and angular scattering properties and their dependences on relative humidity) are used as input parameters to two radiative transfer models (GFDL and University of Michigan) to constrain estimates of aerosol radiative effects, with uncertainties in each step propagated through the analysis. Such comparisons with observations and resultant reductions in uncertainties are

Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing During Boreal Spring

NASA Technical Reports Server (NTRS)

Kim, Maeng-Ki; Lau, K. M.; Chin, Mian; Kim, Kyu-Myong; Sud, Y. C.; Walker, Greg K.

2005-01-01

The direct effects of aerosols on global and regional climate during boreal spring are investigated based on simulations using the NASA Global Modeling and Assimilation Office (GMAO) finite-volume general circulation model (fvGCM) with Microphyics of clouds in Relaxed Arakawa Schubert Scheme (McRAS). The aerosol loading are prescribed from three-dimensional monthly distribution of tropospheric aerosols viz., sulfate, black carbon, organic carbon, soil dust, and sea salt from output of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol extinction coefficient, single scattering albedo, and asymmetric factor are computed as wavelength-dependent radiative forcing in the radiative transfer scheme of the fvGCM, and as a function of the aerosol loading and ambient relative humidity. We find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excites a planetary scale teleconnection pattern in sea level pressure, temperature and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, i.e., South Asia, East Asia, and northern and western Africa. Additionally, atmospheric heating is found in regions with large loading of dust (over Northern Africa, and Middle East), and black carbon (over South-East Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east-west dipole anomaly with strong cooling over the Caspian Sea, and warming over central and northeastern Asia, where aerosol concentration are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes

Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols.

PubMed

Jacobson, M Z

2001-02-08

Aerosols affect the Earth's temperature and climate by altering the radiative properties of the atmosphere. A large positive component of this radiative forcing from aerosols is due to black carbon--soot--that is released from the burning of fossil fuel and biomass, and, to a lesser extent, natural fires, but the exact forcing is affected by how black carbon is mixed with other aerosol constituents. From studies of aerosol radiative forcing, it is known that black carbon can exist in one of several possible mixing states; distinct from other aerosol particles (externally mixed) or incorporated within them (internally mixed), or a black-carbon core could be surrounded by a well mixed shell. But so far it has been assumed that aerosols exist predominantly as an external mixture. Here I simulate the evolution of the chemical composition of aerosols, finding that the mixing state and direct forcing of the black-carbon component approach those of an internal mixture, largely due to coagulation and growth of aerosol particles. This finding implies a higher positive forcing from black carbon than previously thought, suggesting that the warming effect from black carbon may nearly balance the net cooling effect of other anthropogenic aerosol constituents. The magnitude of the direct radiative forcing from black carbon itself exceeds that due to CH4, suggesting that black carbon may be the second most important component of global warming after CO2 in terms of direct forcing.

Host model uncertainties in aerosol radiative forcing estimates: results from the AeroCom prescribed intercomparison study

NASA Astrophysics Data System (ADS)

Stier, P.; Schutgens, N. A. J.; Bian, H.; Boucher, O.; Chin, M.; Ghan, S.; Huneeus, N.; Kinne, S.; Lin, G.; Myhre, G.; Penner, J. E.; Randles, C.; Samset, B.; Schulz, M.; Yu, H.; Zhou, C.

2012-09-01

Simulated multi-model "diversity" in aerosol direct radiative forcing estimates is often perceived as measure of aerosol uncertainty. However, current models used for aerosol radiative forcing calculations vary considerably in model components relevant for forcing calculations and the associated "host-model uncertainties" are generally convoluted with the actual aerosol uncertainty. In this AeroCom Prescribed intercomparison study we systematically isolate and quantify host model uncertainties on aerosol forcing experiments through prescription of identical aerosol radiative properties in nine participating models. Even with prescribed aerosol radiative properties, simulated clear-sky and all-sky aerosol radiative forcings show significant diversity. For a purely scattering case with globally constant optical depth of 0.2, the global-mean all-sky top-of-atmosphere radiative forcing is -4.51 W m-2 and the inter-model standard deviation is 0.70 W m-2, corresponding to a relative standard deviation of 15%. For a case with partially absorbing aerosol with an aerosol optical depth of 0.2 and single scattering albedo of 0.8, the forcing changes to 1.26 W m-2, and the standard deviation increases to 1.21 W m-2, corresponding to a significant relative standard deviation of 96%. However, the top-of-atmosphere forcing variability owing to absorption is low, with relative standard deviations of 9% clear-sky and 12% all-sky. Scaling the forcing standard deviation for a purely scattering case to match the sulfate radiative forcing in the AeroCom Direct Effect experiment, demonstrates that host model uncertainties could explain about half of the overall sulfate forcing diversity of 0.13 W m-2 in the AeroCom Direct Radiative Effect experiment. Host model errors in aerosol radiative forcing are largest in regions of uncertain host model components, such as stratocumulus cloud decks or areas with poorly constrained surface albedos, such as sea ice. Our results demonstrate that host

Host model uncertainties in aerosol radiative forcing estimates: results from the AeroCom Prescribed intercomparison study

NASA Astrophysics Data System (ADS)

Stier, P.; Schutgens, N. A. J.; Bellouin, N.; Bian, H.; Boucher, O.; Chin, M.; Ghan, S.; Huneeus, N.; Kinne, S.; Lin, G.; Ma, X.; Myhre, G.; Penner, J. E.; Randles, C. A.; Samset, B.; Schulz, M.; Takemura, T.; Yu, F.; Yu, H.; Zhou, C.

2013-03-01

Simulated multi-model "diversity" in aerosol direct radiative forcing estimates is often perceived as a measure of aerosol uncertainty. However, current models used for aerosol radiative forcing calculations vary considerably in model components relevant for forcing calculations and the associated "host-model uncertainties" are generally convoluted with the actual aerosol uncertainty. In this AeroCom Prescribed intercomparison study we systematically isolate and quantify host model uncertainties on aerosol forcing experiments through prescription of identical aerosol radiative properties in twelve participating models. Even with prescribed aerosol radiative properties, simulated clear-sky and all-sky aerosol radiative forcings show significant diversity. For a purely scattering case with globally constant optical depth of 0.2, the global-mean all-sky top-of-atmosphere radiative forcing is -4.47 Wm-2 and the inter-model standard deviation is 0.55 Wm-2, corresponding to a relative standard deviation of 12%. For a case with partially absorbing aerosol with an aerosol optical depth of 0.2 and single scattering albedo of 0.8, the forcing changes to 1.04 Wm-2, and the standard deviation increases to 1.01 W-2, corresponding to a significant relative standard deviation of 97%. However, the top-of-atmosphere forcing variability owing to absorption (subtracting the scattering case from the case with scattering and absorption) is low, with absolute (relative) standard deviations of 0.45 Wm-2 (8%) clear-sky and 0.62 Wm-2 (11%) all-sky. Scaling the forcing standard deviation for a purely scattering case to match the sulfate radiative forcing in the AeroCom Direct Effect experiment demonstrates that host model uncertainties could explain about 36% of the overall sulfate forcing diversity of 0.11 Wm-2 in the AeroCom Direct Radiative Effect experiment. Host model errors in aerosol radiative forcing are largest in regions of uncertain host model components, such as stratocumulus

Downscaling Aerosols and the Impact of Neglected Subgrid Processes on Direct Aerosol Radiative Forcing for a Representative Global Climate Model Grid Spacing

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gustafson, William I.; Qian, Yun; Fast, Jerome D.

2011-07-13

Recent improvements to many global climate models include detailed, prognostic aerosol calculations intended to better reproduce the observed climate. However, the trace gas and aerosol fields are treated at the grid-cell scale with no attempt to account for sub-grid impacts on the aerosol fields. This paper begins to quantify the error introduced by the neglected sub-grid variability for the shortwave aerosol radiative forcing for a representative climate model grid spacing of 75 km. An analysis of the value added in downscaling aerosol fields is also presented to give context to the WRF-Chem simulations used for the sub-grid analysis. We foundmore » that 1) the impact of neglected sub-grid variability on the aerosol radiative forcing is strongest in regions of complex topography and complicated flow patterns, and 2) scale-induced differences in emissions contribute strongly to the impact of neglected sub-grid processes on the aerosol radiative forcing. The two of these effects together, when simulated at 75 km vs. 3 km in WRF-Chem, result in an average daytime mean bias of over 30% error in top-of-atmosphere shortwave aerosol radiative forcing for a large percentage of central Mexico during the MILAGRO field campaign.« less

Aerosol Radiative Forcing in Asian Continental Outflow

NASA Technical Reports Server (NTRS)

Pueschel, R.; Kinne, S.; Redemann, J.; Gore, Warren J. (Technical Monitor)

2000-01-01

Aerosols in elevated layers were sampled with FSSP-probes and wire impactors over the Pacific ocean aboard the NASA DC-8 aircraft. Analyses of particle size and morphology identifies two distinctly different aerosol types for cases when the mid-visible extinctions exceed 0.2/km. Smaller sizes (effective radii of 0.2 um) and moderate absorption (mid-visible single scattering albedo of.935) are typical for urban-industrial pollution. Larger sizes (effective radii of 0.7 um) and weak absorption (mid-visible single scattering albedo of 0.985) identify dust. This aerosol classification is in agreement with its origin as determined by airmass back trajectory analysis. Based on lidar vertical profiling, aerosol dominated by dust and urban-industrial pollution above 3km were assigned mid-visible optical depths of 0.50 and 0.27, respectively. Radiative transfer simulations, considering a 50% cloud-cover below the aerosol layers, suggest (on a daily tP C)C> basis) small reductions (-4W/m2) to the energy budget at the top of the atmosphere for both aerosol types. For c' 0 dust, more backscattering of sunlight (weaker solar absorption) is compensated by a stronger greenhouse effect due to larger sizes. Forced reductions to the energy budget at the surface are 12W/m2 for both aerosol types. In contrast, impacts on heating rates within the aerosol layers are quite different: While urban-industrial aerosol warms the layer (at +0.6K/day as solar heating dominates), dust cools (at -0.5K/day as infrared cooling dominates). Sensitivity tests show the dependence of the aerosol climatic impact on the optical depth, particle size, absorptivity, and altitude of the layers, as well as clouds and surface properties. Climatic cooling can be eliminated (1) for the urban-industrial aerosol if absorption is increased to yield a mid-visible single scattering albedo of 0.89, or if the ocean is replaced by a land surface; (2) for the dust aerosol if the effective radius is increased from 0.7 to 1

A Strategy to Assess Aerosol Direct Radiative Forcing of Climate Using Satellite Radiation Measurements

NASA Technical Reports Server (NTRS)

Kaufman, Yoram J.; Tanre, Didier; Einaudi, Franco (Technical Monitor)

2001-01-01

Atmospheric aerosols have a complex internal chemical composition and optical properties. Therefore it is difficult to model their impact on redistribution and absorption of solar radiation, and the consequent impact on atmospheric dynamics and climate. The use in climate models of isolated aerosol parameters retrieved from satellite data (e.g. optical thickness) may result in inconsistent calculations, if the model assumptions differ from these of the satellite retrieval schemes. Here we suggest a strategy to assess the direct impact of aerosol on the radiation budget at the top and bottom of the atmosphere using satellite and ground based measurements of the spectral solar radiation scattered by the aerosol. This method ensures consistent use of the satellite data and increases its accuracy. For Kaufman and Tanre: Strategy for aerosol direct forcing anthropogenic aerosol in the fine mode (e.g. biomass burning smoke and urban pollution) consistent use of satellite derived optical thickness can yield the aerosol impact on the spectral solar flux with accuracy an order of magnitude better than the optical thickness itself. For example, a simulated monthly average smoke optical thickness of 0.5 at 0.55 microns (forcing of 40-50 W/sq m) derived with an error of 20%, while the forcing can be measured directly with an error of only 0-2 W/sq m. Another example, the effect of large dust particles on reflection of solar flux can be derived three times better than retrievals of optical thickness. Since aerosol impacts not only the top of the atmosphere but also the surface irradiation, a combination of satellite and ground based measurements of the spectral flux, can be the most direct mechanism to evaluate the aerosol effect on climate and assimilate it in climate models. The strategy is applied to measurements from SCAR-B and the Tarfox experiments. In SCAR-B aircraft spectral data are used to derive the 24 hour radiative forcing of smoke at the top of the atmosphere of

Aerosol chemistry and the effect of aerosol water content on visibility impairment and radiative forcing in Guangzhou during the 2006 Pearl River Delta campaign.

PubMed

Jung, Jinsang; Lee, Hanlim; Kim, Young J; Liu, Xingang; Zhang, Yuanhang; Gu, Jianwei; Fan, Shaojia

2009-08-01

Optical and chemical aerosol measurements were obtained from 2 to 31 July 2006 at an urban site in the metropolitan area of Guangzhou (China) as part of the Program of Regional Integrated Experiment of Air Quality over Pearl River Delta (PRIDE-PRD2006) to investigate aerosol chemistry and the effect of aerosol water content on visibility impairment and radiative forcing. During the PRIDE-PRD2006 campaign, the average contributions of ammonium sulfate, organic mass by carbon (OMC), elemental carbon (EC), and sea salt (SS) to total PM(2.5) mass were measured to be 36.5%, 5.7%, 27.1%, 7.8%, and 3.7%, respectively. Compared with the clean marine period, (NH(4))(2)SO(4), NH(4)NO(3), and OMC were all greatly enhanced (by up to 430%) during local haze periods via the accumulation of a secondary aerosol component. The OMC dominance increased when high levels of biomass burning influenced the measurement site while (NH(4))(2)SO(4) and OMC did when both biomass burning and industrial emissions influenced it. The effect of aerosol water content on the total light-extinction coefficient was estimated to be 34.2%, of which 25.8% was due to aerosol water in (NH(4))(2)SO(4), 5.1% that in NH(4)NO(3), and 3.3% that in SS. The average mass-scattering efficiency (MSE) of PM(10) particles was determined to be 2.2+/-0.6 and 4.6+/-1.7m(2)g(-1) under dry (RH<40%) and ambient conditions, respectively. The average single-scattering albedo (SSA) was 0.80+/-0.08 and 0.90+/-0.04 under dry and ambient conditions, respectively. Not only are the extinction and scattering coefficients greatly enhanced by aerosol water content, but MSE and SSA are also highly sensitive. It can be concluded that sulfate and carbonaceous aerosol, as well as aerosol water content, play important roles in the processes that determine visibility impairment and radiative forcing in the ambient atmosphere of the Guangzhou urban area.

Anthropogenic aerosol optical and radiative properties in the typical urban/suburban regions in China

NASA Astrophysics Data System (ADS)

Gong, Chongshui; Xin, Jinyuan; Wang, Shigong; Wang, Yuesi; Zhang, Tiejun

2017-11-01

The effect of high anthropogenic aerosols on the aerosol optical and radiative properties was aggravated from west to east in China. The annual mean (from 2004 to 2007) aerosol optical depth (AOD), Ångström exponents (α), absorptive aerosol optical depth (AAOD), and single-scattering albedo (SSA) were from 0.16 to 0.73, from - 0.01 to 1.15, from 0.03 to 0.04, and from 0.78 to 0.94, respectively. In addition, the annual mean of aerosol direct radiative forcing at the top of the atmosphere (TOA) were from - 7.2 to 18.5 W/m2. High anthropogenic aerosol exhibited the effect of heating the atmosphere (ATM) (48-52 W/m2) and cooling the surface (SFC) (- 48 to - 56 W/m2) in eastern China. In Lanzhou where there is more serious pollution of heavy industry, aerosol-induced surface cooling reached - 61 W/m2. The radiative forcing was higher in winter and spring than that in summer and autumn. Aerosol heating effect on the atmosphere was obvious; there was significantly linear correlation between AOD and TOA, SSA and TOA. The slopes of AOD vs TOA were from - 20.8 to - 42.6. The slopes of SSA vs TOA were from - 58 to - 302. The aerosol was cooling the Earth-atmosphere system with AOD or SSA increasing. In the meantime, AAOD (x) exhibited significantly linear correlation with the heating effect in the atmosphere (ATM: y) (y = 1053.7x + 10.5, R2 = 0.85). And the effect of AOD (x) on the SFC (y) cooling was also obvious (y = - 47.1x - 24.5, R2 = 0.56). Therefore, the thermodynamic effects of anthropogenic aerosols on the atmosphere circulation and structure should be taken into consideration in East Asia.

Sensitivity of clear-sky direct radiative effect of the aerosol to micro-physical properties by using 6SV radiative transfer model: preliminary results

NASA Astrophysics Data System (ADS)

Bassani, Cristiana; Tirelli, Cecilia; Manzo, Ciro; Pietrodangelo, Adriana; Curci, Gabriele

2015-04-01

The aerosol micro-physical properties are crucial to analyze their radiative impact on the Earth's radiation budget [IPCC, 2007]. The 6SV model, last generation of the Second Simulation of a Satellite Signal in the Solar Spectrum (6S) radiative transfer code [Kotchenova et al., 2007; Vermote et al., 1997] has been used to perform physically-based atmospheric correction of hyperspectral airborne and aircraft remote sensing data [Vermote et al., 2009; Bassani et al. 2010; Tirelli et al., 2014]. The atmospheric correction of hyperspectral data has been shown to be sensitive to the aerosol micro-physical properties, as reported in Bassani et al., 2012. The role of the aerosol micro-physical properties on the accuracy of the atmospheric correction of hyperspectral data acquired over water and land targets is investigated within the framework of CLAM-PHYM (Coasts and Lake Assessment and Monitoring by PRISMA HYperspectral Mission) and PRIMES (Synergistic use of PRISMA products with high resolution meteo-chemical simulations and their validation on ground and from satellite) projects, both funded by Italian Space Agency (ASI). In this work, the results of the radiative field of the Earth/Atmosphere coupled system simulated by using 6SV during the atmospheric correction of hyperspectral data are presented. The analysis of the clear-sky direct radiative effect is performed considering the aerosol micro-physical properties used to define the aerosol model during the atmospheric correction process. In particular, the AERONET [Holben et al., 1998] and FLEXAOD [Curci et al., 2014] micro-physical properties are used for each image to evaluate the contribution of the size distribution and refractive index of the aerosol type on the surface reflectance and on the direct radiative forcing. The results highlight the potential of the hyperspectral remote sensing data for atmospheric studies as well as for environmental studies. Currently, the future hyperspectral missions, such as the

Response of heterogeneous vegetation to aerosol radiative forcing over a northeast Indian station.

PubMed

Latha, R; Vinayak, B; Murthy, B S

2018-01-15

Importance of atmospheric aerosols through direct and indirect effects on hydrological cycle is highlighted through multiple studies. This study tries to find how much the aerosols can affect evapo-transpiration (ET), a key component of the hydrological cycle over high NDVI (normalized difference vegetation index)/dense canopy, over Dibrugarh, known for vast tea plantation. The radiative effects of aerosols are calculated using satellite (Terra-MODIS) and reanalysis data on daily and monthly scales. Aerosol optical depth (AOD) obtained from satellite and ground observations compares well. Aerosol radiative forcing (ARF), calculated using MERRA data sets of 'clean-clear radiation' and 'clear-radiation' at the surface, shows a lower forcing efficiency, 35 Wm -zs , that is about half of that of ground observations. As vegetation controls ET over high NDVI area to the maximum and that gets modified through ARF, a regression equation is fitted between ET, AOD and NDVI for this station as ET = 0.25 + (-84.27) × AOD + (131.51) × NDVI that explains 82% of 'daily' ET variation using easily available satellite data. ET is found to follow net radiation closely and the direct relation between soil moisture and ET is weak on daily scale over this station as it may be acting through NDVI. Copyright © 2017 Elsevier Ltd. All rights reserved.

Elevated Aerosol Layers and Their Radiative Impact over Kanpur During Monsoon Onset Period

NASA Technical Reports Server (NTRS)

Sarangi, Chandan; Tripathi, S. N.; Mishra, A. K.; Welton, E. J.

2016-01-01

Accurate information about aerosol vertical distribution is needed to reduce uncertainties in aerosol radiative forcing and its effect on atmospheric dynamics. The present study deals with synergistic analyses of aerosol vertical distribution and aerosol optical depth (AOD) with meteorological variables using multisatellite and ground-based remote sensors over Kanpur in central Indo-Gangetic Plain (IGP). Micro-Pulse Lidar Network-derived aerosol vertical extinction (sigma) profiles are analyzed to quantify the interannual and daytime variations during monsoon onset period (May-June) for 2009-2011. The mean aerosol profile is broadly categorized into two layers viz., a surface layer (SL) extending up to 1.5 km (where sigma decreased exponentially with height) and an elevated aerosol layer (EAL) extending between 1.5 and 5.5 km. The increase in total columnar aerosol loading is associated with relatively higher increase in contribution from EAL loading than that from SL. The mean contributions of EALs are about 60%, 51%, and 50% to total columnar AOD during 2009, 2010, and 2011, respectively. We observe distinct parabolic EALs during early morning and late evening but uniformly mixed EALs during midday. The interannual and daytime variations of EALs are mainly influenced by long-range transport and convective capacity of the local emissions, respectively. Radiative flux analysis shows that clear-sky incoming solar radiation at surface is reduced with increase in AOD, which indicates significant cooling at surface. Collocated analysis of atmospheric temperature and aerosol loading reveals that increase in AOD not only resulted in surface dimming but also reduced the temperature (approximately 2-3 C) of lower troposphere (below 3 km altitude). Radiative transfer simulations indicate that the reduction of incoming solar radiation at surface is mainly due to increased absorption by EALs (with increase in total AOD). The observed cooling in lower troposphere in high

A Novel Method for Estimating Shortwave Direct Radiative Effect of Above-cloud Aerosols over Ocean Using CALIOP and MODIS Data

NASA Technical Reports Server (NTRS)

Zhang, Z.; Meyer, K.; Platnick, S.; Oreopoulos, L.; Lee, D.; Yu, H.

2013-01-01

This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It accounts for the overlapping of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure. Effects of sub-grid scale cloud and aerosol variations on DRE are accounted for. It is computationally efficient through using grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table in radiative transfer calculations. We verified that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous shortwave DRE that generally agrees with more rigorous pixel-level computation within 4%. We have also computed the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global ocean based on 4 yr of CALIOP and MODIS data. We found that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds.

Aerosol direct effect on solar radiation over the eastern Mediterranean Sea based on AVHRR satellite measurements

NASA Astrophysics Data System (ADS)

Georgakaki, Paraskevi; Papadimas, Christos D.; Hatzianastassiou, Nikos; Fotiadi, Aggeliki; Matsoukas, Christos; Stackhouse, Paul; Kanakidou, Maria; Vardavas, Ilias M.

2017-04-01

Despite the improved scientific understanding of the direct effect of aerosols on solar radiation (direct radiative effect, DRE) improvements are necessary, for example regarding the accuracy of the magnitude of estimated DREs and their spatial and temporal variability. This variability cannot be ensured by in-situ surface and airborne measurements, while it is also relatively difficult to capture through satellite observations. This becomes even more difficult when complete spatial coverage of extended areas is required, especially concerning areas that host various aerosol types with variable physico-chemical and optical aerosol properties. Better assessments of aerosol DREs are necessary, relying on aerosol optical properties with high spatial and temporal variation. The present study aims to provide a refined, along these lines, assessment of aerosol DREs over the eastern Mediterranean (EM) Sea, which is a key area for aerosol studies. Daily DREs are computed for 1˚ x1˚ latitude-longitude grids with the FORTH detailed spectral radiation transfer model (RTM) using input data for various atmospheric and surface parameters, such as clouds, water vapor, ozone and surface albedo, taken from the NASA-Langley Global Earth Observing System (GEOS) database. The model spectral aerosol optical depth (AOD), single scattering albedo and asymmetry parameter are taken from the Global Aerosol Data Set and the NOAA Climate Data Record (CDR) version 2 of Advanced Very High resolution Radiometer (AVHRR) AOD dataset which is available over oceans at 0.63 microns and at 0.1˚ x0.1˚ . The aerosol DREs are computed at the surface, the top-of-atmosphere and within the atmosphere, over the period 1985-1995. Preliminary model results for the period 1990-1993 reveal a significant spatial and temporal variability of DREs over the EM Sea, for example larger values over the Aegean and Black Seas, surrounded by land areas with significant anthropogenic aerosol sources, and over the

Transport of Aerosols from Asia and Their Radiative Effects Over the Western Pacific: A 3-D Model Study for ACE-Asia Experiment During Spring 2001

NASA Technical Reports Server (NTRS)

Chin, Mian; Ginoux, Paul; Flatau, Piotr; Anderson, Tad; Masonis, Sarah; Russell, Phil; Schmid, Beat; Livingston, John; Redemann, Jens; Kahn, Ralph;

Influence of aerosols on surface reaching spectral irradiance and introduction to a new technique for estimating aerosol radiative forcing from spectral flux measurements

NASA Astrophysics Data System (ADS)

Rao, R. R.

2015-12-01

Aerosol radiative forcing estimates with high certainty are required in climate change studies. The approach in estimating the aerosol radiative forcing by using the chemical composition of aerosols is not effective as the chemical composition data with radiative properties are not widely available. In this study we look into the approach where ground based spectral radiation flux measurements along with an RT model is used to estimate radiative forcing. Measurements of spectral flux were made using an ASD spectroradiometer with 350 - 1050 nm wavelength range and 3nm resolution for around 54 clear-sky days during which AOD range was around 0.1 to 0.7. Simultaneous measurements of black carbon were also made using Aethalometer (Magee Scientific) which ranged from around 1.5 ug/m3 to 8 ug/m3. All the measurements were made in the campus of Indian Institute of Science which is in the heart of Bangalore city. The primary study involved in understanding the sensitivity of spectral flux to change in the mass concentration of individual aerosol species (Optical properties of Aerosols and Clouds -OPAC classified aerosol species) using the SBDART RT model. This made us clearly distinguish the region of influence of different aerosol species on the spectral flux. Following this, a new technique has been introduced to estimate an optically equivalent mixture of aerosol species for the given location. The new method involves an iterative process where the mixture of aerosol species are changed in OPAC model and RT model is run as long as the mixture which mimics the measured spectral flux within 2-3% deviation from measured spectral flux is obtained. Using the optically equivalent aerosol mixture and RT model aerosol radiative forcing is estimated. The new method is limited to clear sky scenes and its accuracy to derive an optically equivalent aerosol mixture reduces when diffuse component of flux increases. Our analysis also showed that direct component of spectral flux is

Observed Reduction In Surface Solar Radiation - Aerosol Forcing Versus Cloud Feedback?

NASA Astrophysics Data System (ADS)

Liepert, B.

The solar radiation reaching the ground is a key parameter for the climate system. It drives the hydrological cycle and numerous biological processes. Surface solar radi- ation revealed an estimated 7W/m2 or 4% decline at sites worldwide from 1961 to 1990. The strongest decline occurred at the United States sites with 19W/m2 or 10%. Increasing air pollution and hence direct and indirect aerosol effect, as we know today can only explain part of the reduction in solar radiation. Increasing cloud optical thick- ness - possibly due to global warming - is a more likely explanation for the observed reduction in solar radiation in the United States. The analysis of surface solar radiation data will be shown and compared with GCM results of the direct and indirect aerosol effect. It will be argued that the residual declines in surface solar radiation is likely due to cloud feedback.

Radiative Forcing of the Pinatubo Aerosol as a Function of Latitude and Time

NASA Technical Reports Server (NTRS)

Bergstrom, R. W.; Kinne, S.; Russell, P. B.; Bauman, J. J.; Minnis, P.

1996-01-01

We present calculations of the radiative forcing of the Mt. Pinatubo aerosols as a function of latitude and time after the eruption and compare the results with GOES satellite data. The results from the model indicate that the net effect of the aerosol was to cool the earth-atmosphere system with the most significant radiative effect in the tropics (corresponding to the location of the tropical stratospheric reservoir) and at latitudes greater than 60 deg. The high-latitude maximum is a combined effect of the high-latitude peak in optical depth (Trepte et al 1994) and the large solar zenith angles. The comparison of the predicted and measured net flux shows relatively good agreement, with the model consistently under predicting the cooling effect of the aerosol.

Radiative Forcing of the Pinatubo Aerosol as a Function of Latitude and Time

NASA Technical Reports Server (NTRS)

Bergstrom, Robert W.; Kinne, S.; Russell, P. B.; Bauman, J. J.; Minnis, P.

2000-01-01

We present calculations of the radiative forcing of the Mt. Pinatubo aerosols as a function of latitude and time after the eruption and compare the results with GOES satellite data. The results from the model indicate that the net effect of the aerosol was to cool the earth-atmosphere system with the most significant radiative effect in the tropics (corresponding to the location of the tropical stratospheric reservoir) and at latitudes greater than 60 degrees. The high-latitude maximum is a combined effect of the high-latitude peak in optical depth (Trepte et al 1994) and the large solar zenith angles. The comparison of the predicted and measured net flux shows relatively good agreement, with the model consistently under predicting the cooling effect of the aerosol.

Observations of enhanced aerosol longwave radiative forcing over an urban environment

NASA Astrophysics Data System (ADS)

Panicker, A. S.; Pandithurai, G.; Safai, P. D.; Kewat, S.

2008-02-01

Collocated measurements of sun/sky radiance, aerosol chemical composition and radiative fluxes have been utilized to estimate longwave aerosol radiative forcing over Pune, an Indian urban site during dry winter [Dec2004 to Feb2005] by two methods. Hybrid method which uses observed downwelling and modeled upwelling longwave fluxes for different aerosol loadings yielded a surface forcing of 9.4 Wm-2. Model approach includes utilization of skyradiometer derived spectral aerosol optical properties in the visible and near infra-red wavelengths, modeled aerosol properties in 1.2-40 μm using observed soot and chemical composition data, MODIS water vapor and TOMS column ozone in a radiative transfer model. Estimates from model method showed longwave enhancement of 6.5 and 8.2 Wm-2 at the surface with tropical model atmosphere and temporally varying profiles of temperature and humidity, respectively. Study reveals that about 25% of the aerosol shortwave cooling is being compensated by increase in longwave radiation due to aerosol absorption.

Aerosol direct radiative effects over the northwest Atlantic, northwest Pacific, and North Indian Oceans: estimates based on in-situ chemical and optical measurements and chemical transport modeling

NASA Astrophysics Data System (ADS)

Bates, T. S.; Anderson, T. L.; Baynard, T.; Bond, T.; Boucher, O.; Carmichael, G.; Clarke, A.; Erlick, C.; Guo, H.; Horowitz, L.; Howell, S.; Kulkarni, S.; Maring, H.; McComiskey, A.; Middlebrook, A.; Noone, K.; O'Dowd, C. D.; Ogren, J.; Penner, J.; Quinn, P. K.; Ravishankara, A. R.; Savoie, D. L.; Schwartz, S. E.; Shinozuka, Y.; Tang, Y.; Weber, R. J.; Wu, Y.

2006-01-01

The largest uncertainty in the radiative forcing of climate change over the industrial era is that due to aerosols, a substantial fraction of which is the uncertainty associated with scattering and absorption of shortwave (solar) radiation by anthropogenic aerosols in cloud-free conditions (IPCC, 2001). Quantifying and reducing the uncertainty in aerosol influences on climate is critical to understanding climate change over the industrial period and to improving predictions of future climate change for assumed emission scenarios. Measurements of aerosol properties during major field campaigns in several regions of the globe during the past decade are contributing to an enhanced understanding of atmospheric aerosols and their effects on light scattering and climate. The present study, which focuses on three regions downwind of major urban/population centers (North Indian Ocean (NIO) during INDOEX, the Northwest Pacific Ocean (NWP) during ACE-Asia, and the Northwest Atlantic Ocean (NWA) during ICARTT), incorporates understanding gained from field observations of aerosol distributions and properties into calculations of perturbations in radiative fluxes due to these aerosols. This study evaluates the current state of observations and of two chemical transport models (STEM and MOZART). Measurements of burdens, extinction optical depth (AOD), and direct radiative effect of aerosols (DRE - change in radiative flux due to total aerosols) are used as measurement-model check points to assess uncertainties. In-situ measured and remotely sensed aerosol properties for each region (mixing state, mass scattering efficiency, single scattering albedo, and angular scattering properties and their dependences on relative humidity) are used as input parameters to two radiative transfer models (GFDL and University of Michigan) to constrain estimates of aerosol radiative effects, with uncertainties in each step propagated through the analysis. Constraining the radiative transfer

Aerosol nucleation and its role for clouds and Earth's radiative forcing in the aerosol-climate model ECHAM5-HAM

NASA Astrophysics Data System (ADS)

Kazil, J.; Stier, P.; Zhang, K.; Quaas, J.; Kinne, S.; O'Donnell, D.; Rast, S.; Esch, M.; Ferrachat, S.; Lohmann, U.; Feichter, J.

2010-05-01

Nucleation from the gas phase is an important source of aerosol particles in the Earth's atmosphere, contributing to the number of cloud condensation nuclei, which form cloud droplets. We have implemented in the aerosol-climate model ECHAM5-HAM a new scheme for neutral and charged nucleation of sulfuric acid and water based on laboratory data, and nucleation of an organic compound and sulfuric acid using a parametrization of cluster activation based on field measurements. We give details of the implementation, compare results with observations, and investigate the role of the individual aerosol nucleation mechanisms for clouds and the Earth's radiative budget. The results of our simulations are most consistent with observations when neutral and charged nucleation of sulfuric acid proceed throughout the troposphere and nucleation due to cluster activation is limited to the forested boundary layer. The globally averaged annual mean contributions of the individual nucleation processes to total absorbed solar short-wave radiation via the direct, semi-direct, indirect cloud-albedo and cloud-lifetime effects in our simulations are -1.15 W/m2 for charged H2SO4/H2O nucleation, -0.235 W/m2 for cluster activation, and -0.05 W/m2 for neutral H2SO4/H2O nucleation. The overall effect of nucleation is -2.55 W/m2, which exceeds the sum of the individual terms due to feedbacks and interactions in the model. Aerosol nucleation contributes over the oceans with -2.18 W/m2 to total absorbed solar short-wave radiation, compared to -0.37 W/m2 over land. We explain the higher effect of aerosol nucleation on Earth's radiative budget over the oceans with the larger area covered by ocean clouds, due to the larger contrast in albedo between clouds and the ocean surface compared to continents, and the larger susceptibility of pristine clouds owing to the saturation of effects. The large effect of charged nucleation in our simulations is not in contradiction with small effects seen in local

Aerosol nucleation and its role for clouds and Earth's radiative forcing in the aerosol-climate model ECHAM5-HAM

NASA Astrophysics Data System (ADS)

Kazil, J.; Stier, P.; Zhang, K.; Quaas, J.; Kinne, S.; O'Donnell, D.; Rast, S.; Esch, M.; Ferrachat, S.; Lohmann, U.; Feichter, J.

2010-11-01

Nucleation from the gas phase is an important source of aerosol particles in the Earth's atmosphere, contributing to the number of cloud condensation nuclei, which form cloud droplets. We have implemented in the aerosol-climate model ECHAM5-HAM a new scheme for neutral and charged nucleation of sulfuric acid and water based on laboratory data, and nucleation of an organic compound and sulfuric acid using a parametrization of cluster activation based on field measurements. We give details of the implementation, compare results with observations, and investigate the role of the individual aerosol nucleation mechanisms for clouds and the Earth's radiative forcing. The results of our simulations are most consistent with observations when neutral and charged nucleation of sulfuric acid proceed throughout the troposphere and nucleation due to cluster activation is limited to the forested boundary layer. The globally averaged annual mean contributions of the individual nucleation processes to total absorbed solar short-wave radiation via the direct, semi-direct, indirect cloud-albedo and cloud-lifetime effects in our simulations are -1.15 W/m2 for charged H2SO4/H2O nucleation, -0.235 W/m2 for cluster activation, and -0.05 W/m2 for neutral H2SO4/H2O nucleation. The overall effect of nucleation is -2.55 W/m2, which exceeds the sum of the individual terms due to feedbacks and interactions in the model. Aerosol nucleation contributes over the oceans with -2.18 W/m2 to total absorbed solar short-wave radiation, compared to -0.37 W/m2 over land. We explain the higher effect of aerosol nucleation on Earth's radiative forcing over the oceans with the larger area covered by ocean clouds, due to the larger contrast in albedo between clouds and the ocean surface compared to continents, and the larger susceptibility of pristine clouds owing to the saturation of effects. The large effect of charged nucleation in our simulations is not in contradiction with small effects seen in local

Assessment of simulated aerosol effective radiative forcings in the terrestrial spectrum

NASA Astrophysics Data System (ADS)

Heyn, Irene; Block, Karoline; Mülmenstädt, Johannes; Gryspeerdt, Edward; Kühne, Philipp; Salzmann, Marc; Quaas, Johannes

2017-01-01

In its fifth assessment report (AR5), the Intergovernmental Panel on Climate Change provides a best estimate of the effective radiative forcing (ERF) due to anthropogenic aerosol at -0.9 W m-2. This value is considerably weaker than the estimate of -1.2 W m-2 in AR4. A part of the difference can be explained by an offset of +0.2 W m-2 which AR5 added to all published estimates that only considered the solar spectrum, in order to account for adjustments in the terrestrial spectrum. We find that, in the CMIP5 multimodel median, the ERF in the terrestrial spectrum is small, unless microphysical effects on ice- and mixed-phase clouds are parameterized. In the latter case it is large but accompanied by a very strong ERF in the solar spectrum. The total adjustments can be separated into microphysical adjustments (aerosol "effects") and thermodynamic adjustments. Using a kernel technique, we quantify the latter and find that the rapid thermodynamic adjustments of water vapor and temperature profiles are small. Observation-based constraints on these model results are urgently needed.

Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States

DOE PAGES

Gan, C.-M.; Pleim, J.; Mathur, R.; ...

2015-11-03

Long-term simulations with the coupled WRF–CMAQ (Weather Research and Forecasting–Community Multi-scale Air Quality) model have been conducted to systematically investigate the changes in anthropogenic emissions of SO 2 and NO x over the past 16 years (1995–2010) across the United States (US), their impacts on anthropogenic aerosol loading over North America, and subsequent impacts on regional radiation budgets. In particular, this study attempts to determine the consequences of the changes in tropospheric aerosol burden arising from substantial reductions in emissions of SO 2 and NO x associated with control measures under the Clean Air Act (CAA) especially on trends inmore » solar radiation. Extensive analyses conducted by Gan et al. (2014a) utilizing observations (e.g., SURFRAD, CASTNET, IMPROVE, and ARM) over the past 16 years (1995–2010) indicate a shortwave (SW) radiation (both all-sky and clear-sky) "brightening" in the US. The relationship of the radiation brightening trend with decreases in the aerosol burden is less apparent in the western US. One of the main reasons for this is that the emission controls under the CAA were aimed primarily at reducing pollutants in areas violating national air quality standards, most of which were located in the eastern US, while the relatively less populated areas in the western US were less polluted at the beginning of this study period. Comparisons of model results with observations of aerosol optical depth (AOD), aerosol concentration, and radiation demonstrate that the coupled WRF–CMAQ model is capable of replicating the trends well even though it tends to underestimate the AOD. In particular, the sulfate concentration predictions were well matched with the observations. The discrepancies found in the clear-sky diffuse SW radiation are likely due to several factors such as the potential increase of ice particles associated with increasing air traffic, the definition of "clear-sky" in the radiation

Assessment of multi-decadal WRF-CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States

DOE PAGES

Gan, C.-M.; Pleim, J.; Mathur, R.; ...

2015-07-01

Multi-decadal simulations with the coupled WRF-CMAQ model have been conducted to systematically investigate the changes in anthropogenic emissions of SO 2 and NO x over the past 21 years (1990–2010) across the United States (US), their impacts on anthropogenic aerosol loading over North America, and subsequent impacts on regional radiation budgets. In particular, this study attempts to determine the consequences of the changes in tropospheric aerosol burden arising from substantial reductions in emissions of SO 2 and NO x associated with control measures under the Clean Air Act (CAA) especially on trends in solar radiation. Extensive analyses conducted by Ganmore » et al. (2014) utilizing observations (e.g. SURFRAD, CASTNET, IMPROVE and ARM) over the past 16 years (1995–2010) indicate a shortwave (SW) radiation (both all-sky and clear-sky) "brightening" in the US. The relationship of the radiation brightening trend with decreases in the aerosol burden is less apparent in the western US. One of the main reasons for this is that the emission controls under the CAA were aimed primarily at reducing pollutants in areas violating national air quality standards, most of which were located in the eastern US while the relatively less populated areas in the western US were less polluted at the beginning of this study period. Comparisons of model results with observations of aerosol optical depth (AOD), aerosol concentration, and radiation demonstrate that the coupled WRF-CMAQ model is capable of replicating the trends well even through it tends to underestimate the AOD. In particular, the sulfate concentration predictions were well matched with the observations. The discrenpancies found in the clear-sky diffuse SW radiation are likely due to several factors such as potential increase of ice particles associated with increasing air traffic, the definition of "clear-sky" in the radiation retrieval methodology and aerosol semi-direct and/or indirect effects which cannot

Assessment of multi-decadal WRF-CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gan, C.-M.; Pleim, J.; Mathur, R.

Multi-decadal simulations with the coupled WRF-CMAQ model have been conducted to systematically investigate the changes in anthropogenic emissions of SO 2 and NO x over the past 21 years (1990–2010) across the United States (US), their impacts on anthropogenic aerosol loading over North America, and subsequent impacts on regional radiation budgets. In particular, this study attempts to determine the consequences of the changes in tropospheric aerosol burden arising from substantial reductions in emissions of SO 2 and NO x associated with control measures under the Clean Air Act (CAA) especially on trends in solar radiation. Extensive analyses conducted by Ganmore » et al. (2014) utilizing observations (e.g. SURFRAD, CASTNET, IMPROVE and ARM) over the past 16 years (1995–2010) indicate a shortwave (SW) radiation (both all-sky and clear-sky) "brightening" in the US. The relationship of the radiation brightening trend with decreases in the aerosol burden is less apparent in the western US. One of the main reasons for this is that the emission controls under the CAA were aimed primarily at reducing pollutants in areas violating national air quality standards, most of which were located in the eastern US while the relatively less populated areas in the western US were less polluted at the beginning of this study period. Comparisons of model results with observations of aerosol optical depth (AOD), aerosol concentration, and radiation demonstrate that the coupled WRF-CMAQ model is capable of replicating the trends well even through it tends to underestimate the AOD. In particular, the sulfate concentration predictions were well matched with the observations. The discrenpancies found in the clear-sky diffuse SW radiation are likely due to several factors such as potential increase of ice particles associated with increasing air traffic, the definition of "clear-sky" in the radiation retrieval methodology and aerosol semi-direct and/or indirect effects which cannot

Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gan, C.-M.; Pleim, J.; Mathur, R.

Long-term simulations with the coupled WRF–CMAQ (Weather Research and Forecasting–Community Multi-scale Air Quality) model have been conducted to systematically investigate the changes in anthropogenic emissions of SO 2 and NO x over the past 16 years (1995–2010) across the United States (US), their impacts on anthropogenic aerosol loading over North America, and subsequent impacts on regional radiation budgets. In particular, this study attempts to determine the consequences of the changes in tropospheric aerosol burden arising from substantial reductions in emissions of SO 2 and NO x associated with control measures under the Clean Air Act (CAA) especially on trends inmore » solar radiation. Extensive analyses conducted by Gan et al. (2014a) utilizing observations (e.g., SURFRAD, CASTNET, IMPROVE, and ARM) over the past 16 years (1995–2010) indicate a shortwave (SW) radiation (both all-sky and clear-sky) "brightening" in the US. The relationship of the radiation brightening trend with decreases in the aerosol burden is less apparent in the western US. One of the main reasons for this is that the emission controls under the CAA were aimed primarily at reducing pollutants in areas violating national air quality standards, most of which were located in the eastern US, while the relatively less populated areas in the western US were less polluted at the beginning of this study period. Comparisons of model results with observations of aerosol optical depth (AOD), aerosol concentration, and radiation demonstrate that the coupled WRF–CMAQ model is capable of replicating the trends well even though it tends to underestimate the AOD. In particular, the sulfate concentration predictions were well matched with the observations. The discrepancies found in the clear-sky diffuse SW radiation are likely due to several factors such as the potential increase of ice particles associated with increasing air traffic, the definition of "clear-sky" in the radiation

Intercomparison of Models Representing Direct Shortwave Radiative Forcing by Sulfate Aerosols

NASA Technical Reports Server (NTRS)

Boucher, O.; Schwartz, S. E.; Ackerman, T. P.; Anderson, T. L.; Bergstrom, B.; Bonnel, B.; Dahlback, A.; Fouquart, Y.; Chylek, P.; Fu, Q.;

Aerosol direct radiative effects over the northwest Atlantic, northwest Pacific, and North Indian Oceans: estimates based on in-situ chemical and optical measurements and chemical transport modeling

NASA Astrophysics Data System (ADS)

Bates, T. S.; Anderson, T. L.; Baynard, T.; Bond, T.; Boucher, O.; Carmichael, G.; Clarke, A.; Erlick, C.; Guo, H.; Horowitz, L.; Howell, S.; Kulkarni, S.; Maring, H.; McComiskey, A.; Middlebrook, A.; Noone, K.; O'Dowd, C. D.; Ogren, J.; Penner, J.; Quinn, P. K.; Ravishankara, A. R.; Savoie, D. L.; Schwartz, S. E.; Shinozuka, Y.; Tang, Y.; Weber, R. J.; Wu, Y.

2006-05-01

The largest uncertainty in the radiative forcing of climate change over the industrial era is that due to aerosols, a substantial fraction of which is the uncertainty associated with scattering and absorption of shortwave (solar) radiation by anthropogenic aerosols in cloud-free conditions (IPCC, 2001). Quantifying and reducing the uncertainty in aerosol influences on climate is critical to understanding climate change over the industrial period and to improving predictions of future climate change for assumed emission scenarios. Measurements of aerosol properties during major field campaigns in several regions of the globe during the past decade are contributing to an enhanced understanding of atmospheric aerosols and their effects on light scattering and climate. The present study, which focuses on three regions downwind of major urban/population centers (North Indian Ocean (NIO) during INDOEX, the Northwest Pacific Ocean (NWP) during ACE-Asia, and the Northwest Atlantic Ocean (NWA) during ICARTT), incorporates understanding gained from field observations of aerosol distributions and properties into calculations of perturbations in radiative fluxes due to these aerosols. This study evaluates the current state of observations and of two chemical transport models (STEM and MOZART). Measurements of burdens, extinction optical depth (AOD), and direct radiative effect of aerosols (DRE - change in radiative flux due to total aerosols) are used as measurement-model check points to assess uncertainties. In-situ measured and remotely sensed aerosol properties for each region (mixing state, mass scattering efficiency, single scattering albedo, and angular scattering properties and their dependences on relative humidity) are used as input parameters to two radiative transfer models (GFDL and University of Michigan) to constrain estimates of aerosol radiative effects, with uncertainties in each step propagated through the analysis. Constraining the radiative transfer

Effects of mixing states on the multiple-scattering properties of soot aerosols.

PubMed

Cheng, Tianhai; Wu, Yu; Gu, Xingfa; Chen, Hao

2015-04-20

The radiative properties of soot aerosols are highly sensitive to the mixing states of black carbon particles and other aerosol components. Light absorption properties are enhanced by the mixing state of soot aerosols. Quantification of the effects of mixing states on the scattering properties of soot aerosol are still not completely resolved, especially for multiple-scattering properties. This study focuses on the effects of the mixing state on the multiple scattering of soot aerosols using the vector radiative transfer model. Two types of soot aerosols with different mixing states such as external mixture soot aerosols and internal mixture soot aerosols are studied. Upward radiance/polarization and hemispheric flux are studied with variable soot aerosol loadings for clear and haze scenarios. Our study showed dramatic changes in upward radiance/polarization due to the effects of the mixing state on the multiple scattering of soot aerosols. The relative difference in upward radiance due to the different mixing states can reach 16%, whereas the relative difference of upward polarization can reach 200%. The effects of the mixing state on the multiple-scattering properties of soot aerosols increase with increasing soot aerosol loading. The effects of the soot aerosol mixing state on upwelling hemispheric flux are much smaller than in upward radiance/polarization, which increase with increasing solar zenith angle. The relative difference in upwelling hemispheric flux due to the different soot aerosol mixing states can reach 18% when the solar zenith angle is 75°. The findings should improve our understanding of the effects of mixing states on the optical properties of soot aerosols and their effects on climate. The mixing mechanism of soot aerosols is of critical importance in evaluating the climate effects of soot aerosols, which should be explicitly included in radiative forcing models and aerosol remote sensing.

The Atmospheric Radiation Measurement Program May 2003 Intensive Operations Period Examining Aerosol Properties and Radiative Influences: Preface to Special Section

NASA Technical Reports Server (NTRS)

Ferrare, Richard; Feingold, Graham; Ghan, Steven; Ogren, John; Schmid, Beat; Schwartz, Stephen E.; Sheridan, Pat

2006-01-01

Atmospheric aerosols influence climate by scattering and absorbing radiation in clear air (direct effects) and by serving as cloud condensation nuclei, modifying the microphysical properties of clouds, influencing radiation and precipitation development (indirect effects). Much of present uncertainty in forcing of climate change is due to uncertainty in the relations between aerosol microphysical and optical properties and their radiative influences (direct effects) and between microphysical properties and their ability to serve as cloud condensation nuclei at given supersaturations (indirect effects). This paper introduces a special section that reports on a field campaign conducted at the Department of Energy Atmospheric Radiation Measurement site in North Central Oklahoma in May, 2003, examining these relations using in situ airborne measurements and surface-, airborne-, and space-based remote sensing.

Uncertainties in global aerosols and climate effects due to biofuel emissions

NASA Astrophysics Data System (ADS)

Kodros, J. K.; Scott, C. E.; Farina, S. C.; Lee, Y. H.; L'Orange, C.; Volckens, J.; Pierce, J. R.

2015-04-01

Aerosol emissions from biofuel combustion impact both health and climate; however, while reducing emissions through improvements to combustion technologies will improve health, the net effect on climate is largely unconstrained. In this study, we examine sensitivities in global aerosol concentration, direct radiative climate effect, and cloud-albedo aerosol indirect climate effect to uncertainties in biofuel emission factors, optical mixing-state, and model nucleation and background SOA. We use the Goddard Earth Observing System global chemical-transport model (GEOS-Chem) with TwO Moment Aerosol Sectional (TOMAS) microphysics. The emission factors include: amount, composition, size and hygroscopicity, as well as optical mixing-state properties. We also evaluate emissions from domestic coal use, which is not biofuel but is also frequently emitted from homes. We estimate the direct radiative effect assuming different mixing states (internal, core-shell, and external) with and without absorptive organic aerosol (brown carbon). We find the global-mean direct radiative effect of biofuel emissions ranges from -0.02 to +0.06 W m-2 across all simulation/mixing state combinations with regional effects in source regions ranging from -0.2 to +1.2 W m-2. The global-mean cloud-albedo aerosol indirect effect ranges from +0.01 to -0.02 W m-2 with regional effects in source regions ranging from -1.0 to -0.05 W m-2. The direct radiative effect is strongly dependent on uncertainties in emissions mass, composition, emissions aerosol size distributions and assumed optical mixing state, while the indirect effect is dependent on the emissions mass, emissions aerosol size distribution and the choice of model nucleation and secondary organic aerosol schemes. The sign and magnitude of these effects have a strong regional dependence. We conclude that the climate effects of biofuel aerosols are largely unconstrained, and the overall sign of the aerosol effects is unclear due to uncertainties

A Global Model Simulation of Aerosol Effects of Surface Radiation Budget- Toward Understanding of the "Dimming to Brightening" Transition

NASA Technical Reports Server (NTRS)

Chin, Mian; Diehl, Thomas; Bian, Huisheng; Yu, Hongbin

2008-01-01

We present a global model study on the role aerosols play in the change of solar radiation at Earth's surface that transitioned from a decreasing (dimming) trend to an increasing (brightening) trend. Our primary objective is to understand the relationship between the long-term trends of aerosol emission, atmospheric burden, and surface solar radiation. More specifically, we use the recently compiled comprehensive global emission datasets of aerosols and precursors from fuel combustion, biomass burning, volcanic eruptions and other sources from 1980 to 2006 to simulate long-term variations of aerosol distributions and optical properties, and then calculate the multi-decadal changes of short-wave radiative fluxes at the surface and at the top of the atmosphere by coupling the GOCART model simulated aerosols with the Goddard radiative transfer model. The model results are compared with long-term observational records from ground-based networks and satellite data. We will address the following critical questions: To what extent can the observed surface solar radiation trends, known as the transition from dimming to brightening, be explained by the changes of anthropogenic and natural aerosol loading on global and regional scales? What are the relative contributions of local emission and long-range transport to the surface radiation budget and how do these contributions change with time?

A 3-D Model Study of Aerosol Composition and Radiative Forcing in the Asian-Pacific Region

NASA Technical Reports Server (NTRS)

Chin, Mian; Ginoux, Paul; Torres, Omar; Zhao, Xuepeng; Einaudi, Franco (Technical Monitor)

2000-01-01

The Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model will be used in analyzing the aerosol data in the ACE-Asia program. Our objectives are (1) to understand the physical, chemical, and optical properties of aerosol and the processes that control these properties over the Asian-Pacific region, (2) to determine the aerosol radiative forcing over the Asian-Pacific region, and (3) to investigate the interaction between aerosol and tropospheric chemistry. We will present the GOCART aerosol simulations of sulfate, dust, carbonaceous, and sea salt concentrations, their optical thicknesses, and their radiative effects. We will also show the comparisons of model results with data taken from previous field campaigns, ground-based sun photometer measurements, and satellite observations. Finally, we will present our plan for the ACE-Asia study.

Impacts of global open-fire aerosols on direct radiative, cloud and surface-albedo effects simulated with CAM5

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jiang, Yiquan; Lu, Zheng; Liu, Xiaohong

Aerosols from open-land fires could significantly perturb the global radiation balance and induce climate change. In this study, Community Atmosphere Model version 5 (CAM5) with prescribed daily fire aerosol emissions is used to investigate the spatial and seasonal characteristics of radiative effects (REs, relative to the case of no fires) of open-fire aerosols including black carbon (BC) and particulate organic matter (POM) from 2003 to 2011. The global annual mean RE from aerosol–radiation interactions (REari) of all fire aerosols is 0.16 ± 0.01 W m –2 (1 σ uncertainty), mainly due to the absorption of fire BC (0.25 ± 0.01 Wmore » m –2), while fire POM induces a small effect (–0.05 and 0.04 ± 0.01 W m –2 based on two different methods). Strong positive REari is found in the Arctic and in the oceanic regions west of southern Africa and South America as a result of amplified absorption of fire BC above low-level clouds, in general agreement with satellite observations. The global annual mean RE due to aerosol–cloud interactions (REaci) of all fire aerosols is –0.70 ± 0.05 W m –2, resulting mainly from the fire POM effect (–0.59 ± 0.03 W m –2). REari (0.43 ± 0.03 W m –2) and REaci (–1.38 ± 0.23 W m –2) in the Arctic are stronger than in the tropics (0.17 ± 0.02 and –0.82 ± 0.09 W m –2 for REari and REaci), although the fire aerosol burden is higher in the tropics. The large cloud liquid water path over land areas and low solar zenith angle of the Arctic favor the strong fire aerosol REaci (up to –15 W m –2) during the Arctic summer. Significant surface cooling, precipitation reduction and increasing amounts of low-level cloud are also found in the Arctic summer as a result of the fire aerosol REaci based on the atmosphere-only simulations. Furthermore, the global annual mean RE due to surface-albedo changes (REsac) over land areas (0.030 ± 0.10 W m –2) is small and statistically insignificant and is mainly due to

Impacts of global open-fire aerosols on direct radiative, cloud and surface-albedo effects simulated with CAM5

DOE PAGES

Jiang, Yiquan; Lu, Zheng; Liu, Xiaohong; ...

2016-11-29

Aerosols from open-land fires could significantly perturb the global radiation balance and induce climate change. In this study, Community Atmosphere Model version 5 (CAM5) with prescribed daily fire aerosol emissions is used to investigate the spatial and seasonal characteristics of radiative effects (REs, relative to the case of no fires) of open-fire aerosols including black carbon (BC) and particulate organic matter (POM) from 2003 to 2011. The global annual mean RE from aerosol–radiation interactions (REari) of all fire aerosols is 0.16 ± 0.01 W m –2 (1 σ uncertainty), mainly due to the absorption of fire BC (0.25 ± 0.01 Wmore » m –2), while fire POM induces a small effect (–0.05 and 0.04 ± 0.01 W m –2 based on two different methods). Strong positive REari is found in the Arctic and in the oceanic regions west of southern Africa and South America as a result of amplified absorption of fire BC above low-level clouds, in general agreement with satellite observations. The global annual mean RE due to aerosol–cloud interactions (REaci) of all fire aerosols is –0.70 ± 0.05 W m –2, resulting mainly from the fire POM effect (–0.59 ± 0.03 W m –2). REari (0.43 ± 0.03 W m –2) and REaci (–1.38 ± 0.23 W m –2) in the Arctic are stronger than in the tropics (0.17 ± 0.02 and –0.82 ± 0.09 W m –2 for REari and REaci), although the fire aerosol burden is higher in the tropics. The large cloud liquid water path over land areas and low solar zenith angle of the Arctic favor the strong fire aerosol REaci (up to –15 W m –2) during the Arctic summer. Significant surface cooling, precipitation reduction and increasing amounts of low-level cloud are also found in the Arctic summer as a result of the fire aerosol REaci based on the atmosphere-only simulations. Furthermore, the global annual mean RE due to surface-albedo changes (REsac) over land areas (0.030 ± 0.10 W m –2) is small and statistically insignificant and is mainly due to

Radiative forcing of the direct aerosol effect from AeroCom Phase II simulations

DOE Office of Scientific and Technical Information (OSTI.GOV)

Myhre, G.; Samset, B. H.; Schulz, M.

2013-01-01

We report on the AeroCom Phase II direct aerosol effect (DAE) experiment where 16 detailed global aerosol models have been used to simulate the changes in the aerosol distribution over the industrial era. All 16 models have estimated the radiative forcing (RF) of the anthropogenic DAE, and have taken into account anthropogenic sulphate, black carbon (BC) and organic aerosols (OA) from fossil fuel, biofuel, and biomass burning emissions. In addition several models have simulated the DAE of anthropogenic nitrate and anthropogenic influenced secondary organic aerosols (SOA). The model simulated all-sky RF of the DAE from total anthropogenic aerosols has amore » range from -0.58 to -0.02 Wm -2, with a mean of -0.27 Wm -2 for the 16 models. Several models did not include nitrate or SOA and modifying the estimate by accounting for this with information from the other AeroCom models reduces the range and slightly strengthens the mean. Modifying the model estimates for missing aerosol components and for the time period 1750 to 2010 results in a mean RF for the DAE of -0.35 Wm -2. Compared to AeroCom Phase I (Schulz et al., 2006) we find very similar spreads in both total DAE and aerosol component RF. However, the RF of the total DAE is stronger negative and RF from BC from fossil fuel and biofuel emissions are stronger positive in the present study than in the previous AeroCom study. We find a tendency for models having a strong (positive) BC RF to also have strong (negative) sulphate or OA RF. This relationship leads to smaller uncertainty in the total RF of the DAE compared to the RF of the sum of the individual aerosol components. The spread in results for the individual aerosol components is substantial, and can be divided into diversities in burden, mass extinction coefficient (MEC), and normalized RF with respect to AOD. We find that these three factors give similar contributions to the spread in results.« less

Radiative Forcing of the Direct Aerosol Effect from AeroCom Phase II Simulations

NASA Technical Reports Server (NTRS)

Myhre, G.; Samset, B. H.; Schulz, M.; Balkanski, Y.; Bauer, S.; Berntsen, T. K.; Bian, H.; Bellouin, N.; Chin, M.; Diehl, T.;

Radiative forcing of the direct aerosol effect from AeroCom Phase II simulations

NASA Astrophysics Data System (ADS)

Myhre, G.; Samset, B. H.; Schulz, M.; Balkanski, Y.; Bauer, S.; Berntsen, T. K.; Bian, H.; Bellouin, N.; Chin, M.; Diehl, T.; Easter, R. C.; Feichter, J.; Ghan, S. J.; Hauglustaine, D.; Iversen, T.; Kinne, S.; Kirkevåg, A.; Lamarque, J.-F.; Lin, G.; Liu, X.; Lund, M. T.; Luo, G.; Ma, X.; van Noije, T.; Penner, J. E.; Rasch, P. J.; Ruiz, A.; Seland, Ø.; Skeie, R. B.; Stier, P.; Takemura, T.; Tsigaridis, K.; Wang, P.; Wang, Z.; Xu, L.; Yu, H.; Yu, F.; Yoon, J.-H.; Zhang, K.; Zhang, H.; Zhou, C.

2013-02-01

We report on the AeroCom Phase II direct aerosol effect (DAE) experiment where 16 detailed global aerosol models have been used to simulate the changes in the aerosol distribution over the industrial era. All 16 models have estimated the radiative forcing (RF) of the anthropogenic DAE, and have taken into account anthropogenic sulphate, black carbon (BC) and organic aerosols (OA) from fossil fuel, biofuel, and biomass burning emissions. In addition several models have simulated the DAE of anthropogenic nitrate and anthropogenic influenced secondary organic aerosols (SOA). The model simulated all-sky RF of the DAE from total anthropogenic aerosols has a range from -0.58 to -0.02 Wm-2, with a mean of -0.27 Wm-2 for the 16 models. Several models did not include nitrate or SOA and modifying the estimate by accounting for this with information from the other AeroCom models reduces the range and slightly strengthens the mean. Modifying the model estimates for missing aerosol components and for the time period 1750 to 2010 results in a mean RF for the DAE of -0.35 Wm-2. Compared to AeroCom Phase I (Schulz et al., 2006) we find very similar spreads in both total DAE and aerosol component RF. However, the RF of the total DAE is stronger negative and RF from BC from fossil fuel and biofuel emissions are stronger positive in the present study than in the previous AeroCom study. We find a tendency for models having a strong (positive) BC RF to also have strong (negative) sulphate or OA RF. This relationship leads to smaller uncertainty in the total RF of the DAE compared to the RF of the sum of the individual aerosol components. The spread in results for the individual aerosol components is substantial, and can be divided into diversities in burden, mass extinction coefficient (MEC), and normalized RF with respect to AOD. We find that these three factors give similar contributions to the spread in results.

Radiative forcing of the direct aerosol effect from AeroCom Phase II simulations

NASA Astrophysics Data System (ADS)

Myhre, G.; Samset, B. H.; Schulz, M.; Balkanski, Y.; Bauer, S.; Berntsen, T. K.; Bian, H.; Bellouin, N.; Chin, M.; Diehl, T.; Easter, R. C.; Feichter, J.; Ghan, S. J.; Hauglustaine, D.; Iversen, T.; Kinne, S.; Kirkevåg, A.; Lamarque, J.-F.; Lin, G.; Liu, X.; Luo, G.; Ma, X.; Penner, J. E.; Rasch, P. J.; Seland, Ø.; Skeie, R. B.; Stier, P.; Takemura, T.; Tsigaridis, K.; Wang, Z.; Xu, L.; Yu, H.; Yu, F.; Yoon, J.-H.; Zhang, K.; Zhang, H.; Zhou, C.

2012-08-01

We report on the AeroCom Phase II direct aerosol effect (DAE) experiment where 15 detailed global aerosol models have been used to simulate the changes in the aerosol distribution over the industrial era. All 15 models have estimated the radiative forcing (RF) of the anthropogenic DAE, and have taken into account anthropogenic sulphate, black carbon (BC) and organic aerosols (OA) from fossil fuel, biofuel, and biomass burning emissions. In addition several models have simulated the DAE of anthropogenic nitrate and anthropogenic influenced secondary organic aerosols (SOA). The model simulated all-sky RF of the DAE from total anthropogenic aerosols has a range from -0.58 to -0.02 W m-2, with a mean of -0.30 W m-2 for the 15 models. Several models did not include nitrate or SOA and modifying the estimate by accounting for this with information from the other AeroCom models reduces the range and slightly strengthens the mean. Modifying the model estimates for missing aerosol components and for the time period 1750 to 2010 results in a mean RF for the DAE of -0.39 W m-2. Compared to AeroCom Phase I (Schulz et al., 2006) we find very similar spreads in both total DAE and aerosol component RF. However, the RF of the total DAE is stronger negative and RF from BC from fossil fuel and biofuel emissions are stronger positive in the present study than in the previous AeroCom study. We find a tendency for models having a strong (positive) BC RF to also have strong (negative) sulphate or OA RF. This relationship leads to smaller uncertainty in the total RF of the DAE compared to the RF of the sum of the individual aerosol components. The spread in results for the individual aerosol components is substantial, and can be divided into diversities in burden, mass extinction coefficient (MEC), and normalized RF with respect to AOD. We find that these three factors give similar contributions to the spread in results.

Seasonal variations of aerosol optical properties, vertical distribution and associated radiative effects in the Yangtze Delta Region of China

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Jianjun; Zheng, Youfei; Li, Zhanqing

2012-02-09

Four years of columnar aerosol particle optical properties (2006 to 2009) and one year database worth of aerosol particle vertical profile of 527 nm extinction coefficient (June 2008 to May 2009) are analyzed at Taihu in the central Yangtze Delta region in eastern China. Seasonal variations of aerosol optical properties, vertical distribution, and influence on shortwave radiation and heating rates were investigated. Multiyear variations of aerosol optical depths (AOD), Angstrom exponents, single scattering albedo (SSA) and asymmetry factor (ASY) are analyzed, together with the vertical profile of aerosol extinction. AOD is largest in summer and smallest in winter. SSAs exhibitmore » weak seasonal variation with the smallest values occurring during winter and the largest during summer. The vast majority of aerosol particles are below 2 km, and about 62%, 67%, 67% and 83% are confined to below 1 km in spring, summer, autumn and winter, respectively. Five-day back trajectory analyses show that the some aerosols aloft are traced back to northern/northwestern China, as far as Mongolia and Siberia, in spring, autumn and winter. The presence of dust aerosols were identified based on the linear depolarization measurements together with other information (i.e., back trajectory, precipitation, aerosol index). Dust strongly impacts the vertical particle distribution in spring and autumn, with much smaller effects in winter. The annual mean aerosol direct shortwave radiative forcing (efficiency) at the bottom, top and within the atmosphere are -34.8 {+-} 9.1 (-54.4 {+-} 5.3), -8.2 {+-} 4.8 (-13.1 {+-} 1.5) and 26.7 {+-} 9.4 (41.3 {+-} 4.6) W/m{sup 2} (Wm{sup -2} T{sup -1}), respectively. The mean reduction in direct and diffuse radiation reaching surface amount to 109.2 {+-} 49.4 and 66.8 {+-} 33.3 W/m{sup 2}, respectively. Aerosols significantly alter the vertical profile of solar heating, with great implications for atmospheric stability and dynamics within the lower

Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

DOE Office of Scientific and Technical Information (OSTI.GOV)

Feng, Y.; Kotamarthi, V. R.; Coulter, R.

Aerosol radiative effects and thermodynamic responses over South Asia are examined with the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of aerosol optical depths (AODs) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in northern India. The WRF-Chem model is found to heavily underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model's low bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profilesmore » averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48% more heating in the atmosphere and 21% more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7K day −1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond

Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

DOE Office of Scientific and Technical Information (OSTI.GOV)

Feng, Y.; Kotamarthi, V. R.; Coulter, R.

Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AODmore » and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day −1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond

Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

DOE PAGES

Feng, Y.; Kotamarthi, V. R.; Coulter, R.; ...

2016-01-18

Aerosol radiative effects and thermodynamic responses over South Asia are examined with the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of aerosol optical depths (AODs) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in northern India. The WRF-Chem model is found to heavily underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model's low bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profilesmore » averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48% more heating in the atmosphere and 21% more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7K day −1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond

Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

DOE PAGES

Feng, Y.; Kotamarthi, V. R.; Coulter, R.; ...

2015-06-19

Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AODmore » and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day −1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond

Improvement in Clouds and the Earth's Radiant Energy System/Surface and Atmosphere Radiation Budget Dust Aerosol Properties, Effects on Surface Validation of Clouds and Radiative Swath

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rutan, D.; Rose, F.; Charlock, T.P.

2005-03-18

Within the Clouds and the Earth's Radiant Energy System (CERES) science team (Wielicki et al. 1996), the Surface and Atmospheric Radiation Budget (SARB) group is tasked with calculating vertical profiles of heating rates, globally, and continuously, beneath CERES footprint observations of Top of Atmosphere (TOA) fluxes. This is accomplished using a fast radiative transfer code originally developed by Qiang Fu and Kuo-Nan Liou (Fu and Liou 1993) and subsequently highly modified by the SARB team. Details on the code and its inputs can be found in Kato et al. (2005) and Rose and Charlock (2002). Among the many required inputsmore » is characterization of the vertical column profile of aerosols beneath each footprint. To do this SARB combines aerosol optical depth information from the moderate-resolution imaging spectroradiometer (MODIS) instrument along with aerosol constituents specified by the Model for Atmosphere and Chemical Transport (MATCH) of Collins et al. (2001), and aerosol properties (e.g. single scatter albedo and asymmetry parameter) from Tegen and Lacis (1996) and OPAC (Hess et al. 1998). The publicly available files that include these flux profiles, called the Clouds and Radiative Swath (CRS) data product, available from the Langley Atmospheric Sciences Data Center (http://eosweb.larc.nasa.gov/). As various versions of the code are completed, publishable results are named ''Editions.'' After CRS Edition 2A was finalized it was found that dust aerosols were too absorptive. Dust aerosols have subsequently been modified using a new set of properties developed by Andy Lacis and results have been released in CRS Edition 2B. This paper discusses the effects of changing desert dust aerosol properties, which can be significant for the radiation budget in mid ocean, a few thousand kilometers from the source regions. Resulting changes are validated via comparison of surface observed fluxes from the Saudi Solar Village surface site (Myers et al. 1999), and the E

Daytime variation of aerosol optical depth in North China and its impact on aerosol direct radiative effects

NASA Astrophysics Data System (ADS)

Song, Jingjing; Xia, Xiangao; Che, Huizheng; Wang, Jun; Zhang, Xiaoling; Li, Xiaojing

2018-06-01

Daytime cycles of aerosol optical depth (AOD) and Angstrom exponent (AE) climatology were analyzed based on long-term (5-15 years) measurements at 18 stations of the China Aerosol Remote Sensing Network (CARSNET) in North China. AOD in Northwest China (NWC) exhibits a daytime trend with negative departures in the early morning and later afternoon while positive departures at midday. Daytime AOD relative departure in different sites and seasons varies from -30.26% to 30.28%. AE in NWC shows an opposite pattern to daytime variation of AOD. Daytime variation of AE is negligible in North China Plain (NCP), AOD increases steadily throughout the day. This trend is consistent and repeatable in four seasons. Such pronounced variability in AOD and AE should be taken accounted for in the estimation of diurnal aerosol direct radiative effects (ADRE), as suggested by the radiative transfer model simulations. The replacement of the observed daytime variation of AOD and AE by daytime mean values in NWC results in ADRE differences of 0.31 Wm-2 at the surface and 0.05 Wm-2 at the top of the atmosphere (TOA). ADRE in NWC will be underestimated by -0.47 Wm-2 and -0.25 Wm-2 at the surface and TOA, respectively, if instantaneous AOD and AE during the overpass time of Terra and Aqua are taken as the daytime mean values. The annual mean ADRE at the surface and TOA will be underestimated by -0.17 Wm-2 and -0.03 Wm-2 if daytime variations of AOD and AE are replaced by daytime mean values in NCP. ADRE will be underestimated by -0.07 Wm-2 at the surface and -0.06 Wm-2 at the TOA if instantaneous AOD and AE during the overpass time of Terra and Aqua other than daytime variation of AOD and AE are used in the calculations.

Overview of ACE-Asia Spring 2001 Investigations On Aerosol-Radiation Interactions

NASA Technical Reports Server (NTRS)

Russell, P. B.; Flatau, P. J.; Valero, F. P. J.; Nakajima, T.; Holben, B.; Pilewskie, P.; Bergin, M.; Schmid, B.; Bergstrom, R. W.; Vogelmann, A.;

North Atlantic Aerosol Properties for Radiative Impact Assessments. Derived from Column Closure Analyses in TARFOX and ACE-2

NASA Technical Reports Server (NTRS)

Russell, Philip A.; Bergstrom, Robert A.; Schmid, Beat; Livingston, John M.

2000-01-01

Aerosol effects on atmospheric radiative fluxes provide a forcing function that can change the climate in potentially significant ways. This aerosol radiative forcing is a major source of uncertainty in understanding the climate change of the past century and predicting future climate. To help reduce this uncertainty, the 1996 Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) and the 1997 Aerosol Characterization Experiment (ACE-2) measured the properties and radiative effects of aerosols over the Atlantic Ocean. Both experiments used remote and in situ measurements from aircraft and the surface, coordinated with overpasses by a variety of satellite radiometers. TARFOX focused on the urban-industrial haze plume flowing from the United States over the western Atlantic, whereas ACE-2 studied aerosols over the eastern Atlantic from both Europe and Africa. These aerosols often have a marked impact on satellite-measured radiances. However, accurate derivation of flux changes, or radiative forcing, from the satellite measured radiances or retrieved aerosol optical depths (AODs) remains a difficult challenge. Here we summarize key initial results from TARFOX and ACE-2, with a focus on closure analyses that yield aerosol microphysical models for use in improved assessments of flux changes. We show how one such model gives computed radiative flux sensitivities (dF/dAOD) that agree with values measured in TARFOX and preliminary values computed for the polluted marine boundary layer in ACE-2. A companion paper uses the model to compute aerosol-induced flux changes over the North Atlantic from AVHRR-derived AOD fields.

Uncertainties in global aerosols and climate effects due to biofuel emissions

NASA Astrophysics Data System (ADS)

Kodros, J. K.; Scott, C. E.; Farina, S. C.; Lee, Y. H.; L'Orange, C.; Volckens, J.; Pierce, J. R.

2015-08-01

Aerosol emissions from biofuel combustion impact both health and climate; however, while reducing emissions through improvements to combustion technologies will improve health, the net effect on climate is largely unconstrained. In this study, we examine sensitivities in global aerosol concentration, direct radiative climate effect, and cloud-albedo aerosol indirect climate effect to uncertainties in biofuel emission factors, optical mixing state, and model nucleation and background secondary organic aerosol (SOA). We use the Goddard Earth Observing System global chemical-transport model (GEOS-Chem) with TwO Moment Aerosol Sectional (TOMAS) microphysics. The emission factors include amount, composition, size, and hygroscopicity, as well as optical mixing-state properties. We also evaluate emissions from domestic coal use, which is not biofuel but is also frequently emitted from homes. We estimate the direct radiative effect assuming different mixing states (homogeneous, core-shell, and external) with and without absorptive organic aerosol (brown carbon). We find the global-mean direct radiative effect of biofuel emissions ranges from -0.02 to +0.06 W m-2 across all simulation/mixing-state combinations with regional effects in source regions ranging from -0.2 to +0.8 W m-2. The global-mean cloud-albedo aerosol indirect effect (AIE) ranges from +0.01 to -0.02 W m-2 with regional effects in source regions ranging from -1.0 to -0.05 W m-2. The direct radiative effect is strongly dependent on uncertainties in emissions mass, composition, emissions aerosol size distributions, and assumed optical mixing state, while the indirect effect is dependent on the emissions mass, emissions aerosol size distribution, and the choice of model nucleation and secondary organic aerosol schemes. The sign and magnitude of these effects have a strong regional dependence. We conclude that the climate effects of biofuel aerosols are largely unconstrained, and the overall sign of the aerosol

Aerosol climate change effects on land ecosystem services.

PubMed

Unger, N; Yue, X; Harper, K L

2017-08-24

A coupled global aerosol-carbon-climate model is applied to assess the impacts of aerosol physical climate change on the land ecosystem services gross primary productivity (GPP) and net primary productivity (NPP) in the 1996-2005 period. Aerosol impacts are quantified on an annual mean basis relative to the hypothetical aerosol-free world in 1996-2005, the global climate state in the absence of the historical rise in aerosol pollution. We examine the separate and combined roles of fast feedbacks associated with the land and slow feedbacks associated with the ocean. We consider all fossil fuel, biofuel and biomass burning aerosol emission sources as anthropogenic. The effective radiative forcing for aerosol-radiation interactions is -0.44 W m -2 and aerosol-cloud interactions is -1.64 W m -2 . Aerosols cool and dry the global climate system by -0.8 °C and -0.08 mm per day relative to the aerosol-free world. Without aerosol pollution, human-induced global warming since the preindustrial would have already exceeded the 1.5 °C aspirational limit set in the Paris Agreement by the 1996-2005 decade. Aerosol climate impacts on the global average land ecosystem services are small due to large opposite sign effects in the tropical and boreal biomes. Aerosol slow feedbacks associated with the ocean strongly dominate impacts in the Amazon and North American Boreal. Aerosol cooling of the Amazon by -1.2 °C drives NPP increases of 8% or +0.76 ± 0.61 PgC per year, a 5-10 times larger impact than estimates of diffuse radiation fertilization by biomass burning aerosol in this region. The North American Boreal suffers GPP and NPP decreases of 35% due to aerosol-induced cooling and drying (-1.6 °C, -0.14 mm per day). Aerosol-land feedbacks play a larger role in the eastern US and Central Africa. Our study identifies an eco-climate teleconnection in the polluted earth system: the rise of the northern hemisphere mid-latitude reflective aerosol pollution layer causes long range

Reduced anthropogenic aerosol radiative forcing caused by biogenic new particle formation

PubMed Central

Sengupta, Kamalika; Duplissy, Jonathan; Frege, Carla; Williamson, Christina; Heinritzi, Martin; Simon, Mario; Yan, Chao; Almeida, João; Tröstl, Jasmin; Nieminen, Tuomo; Ortega, Ismael K.; Wagner, Robert; Dunne, Eimear M.; Adamov, Alexey; Amorim, Antonio; Bernhammer, Anne-Kathrin; Bianchi, Federico; Breitenlechner, Martin; Brilke, Sophia; Chen, Xuemeng; Craven, Jill S.; Dias, Antonio; Ehrhart, Sebastian; Fischer, Lukas; Flagan, Richard C.; Franchin, Alessandro; Fuchs, Claudia; Guida, Roberto; Hakala, Jani; Hoyle, Christopher R.; Jokinen, Tuija; Junninen, Heikki; Kangasluoma, Juha; Kim, Jaeseok; Krapf, Manuel; Kürten, Andreas; Laaksonen, Ari; Lehtipalo, Katrianne; Makhmutov, Vladimir; Mathot, Serge; Molteni, Ugo; Monks, Sarah A.; Onnela, Antti; Peräkylä, Otso; Piel, Felix; Petäjä, Tuukka; Praplan, Arnaud P.; Pringle, Kirsty J.; Richards, Nigel A. D.; Rissanen, Matti P.; Rondo, Linda; Sarnela, Nina; Scott, Catherine E.; Seinfeld, John H.; Sharma, Sangeeta; Sipilä, Mikko; Steiner, Gerhard; Stozhkov, Yuri; Stratmann, Frank; Tomé, Antonio; Virtanen, Annele; Vogel, Alexander Lucas; Wagner, Andrea C.; Wagner, Paul E.; Weingartner, Ernest; Wimmer, Daniela; Winkler, Paul M.; Ye, Penglin; Zhang, Xuan; Hansel, Armin; Worsnop, Douglas R.; Baltensperger, Urs; Kulmala, Markku; Curtius, Joachim

2016-01-01

The magnitude of aerosol radiative forcing caused by anthropogenic emissions depends on the baseline state of the atmosphere under pristine preindustrial conditions. Measurements show that particle formation in atmospheric conditions can occur solely from biogenic vapors. Here, we evaluate the potential effect of this source of particles on preindustrial cloud condensation nuclei (CCN) concentrations and aerosol–cloud radiative forcing over the industrial period. Model simulations show that the pure biogenic particle formation mechanism has a much larger relative effect on CCN concentrations in the preindustrial atmosphere than in the present atmosphere because of the lower aerosol concentrations. Consequently, preindustrial cloud albedo is increased more than under present day conditions, and therefore the cooling forcing of anthropogenic aerosols is reduced. The mechanism increases CCN concentrations by 20–100% over a large fraction of the preindustrial lower atmosphere, and the magnitude of annual global mean radiative forcing caused by changes of cloud albedo since 1750 is reduced by 0.22 W m−2 (27%) to −0.60 W m−2. Model uncertainties, relatively slow formation rates, and limited available ambient measurements make it difficult to establish the significance of a mechanism that has its dominant effect under preindustrial conditions. Our simulations predict more particle formation in the Amazon than is observed. However, the first observation of pure organic nucleation has now been reported for the free troposphere. Given the potentially significant effect on anthropogenic forcing, effort should be made to better understand such naturally driven aerosol processes. PMID:27790989

Interpreting the Ultraviolet Aerosol Index Observed with the OMI Satellite Instrument to Understand Absorption by Organic Aerosols: Implications for Atmospheric Oxidation and Direct Radiative Effects

NASA Technical Reports Server (NTRS)

Hammer, Melanie S.; Martin, Randall V.; Donkelaar, Aaron van; Buchard, Virginie; Torres, Omar; Ridley, David A.; Spurr, Robert J. D.

2016-01-01

Satellite observations of the ultraviolet aerosol index (UVAI) are sensitive to absorption of solar radiation by aerosols; this absorption affects photolysis frequencies and radiative forcing. We develop a global simulation of the UVAI using the 3-D chemical transport model GEOSChem coupled with the Vector Linearized Discrete Ordinate Radiative Transfer model (VLIDORT). The simulation is applied to interpret UVAI observations from the Ozone Monitoring Instrument (OMI) for the year 2007. Simulated and observed values are highly consistent in regions where mineral dust dominates the UVAI, but a large negative bias (-0.32 to -0.97) exists between simulated and observed values in biomass burning regions. We determine effective optical properties for absorbing organic aerosol, known as brown carbon (BrC), and implement them into GEOS-Chem to better represent observed UVAI values over biomass burning regions. The inclusion of absorbing BrC decreases the mean bias between simulated and OMI UVAI values from -0.57 to -0.09 over West Africa in January, from -0.32 to +0.0002 over South Asia in April, from -0.97 to -0.22 over southern Africa in July, and from -0.50 to +0.33 over South America in September. The spectral dependence of absorption after including BrC in the model is broadly consistent with reported observations for biomass burning aerosol, with absorbing Angstrom exponent (AAE) values ranging from 2.9 in the ultraviolet (UV) to 1.3 across the UV-Near IR spectrum. We assess the effect of the additional UV absorption by BrC on atmospheric photochemistry by examining tropospheric hydroxyl radical (OH) concentrations in GEOS-Chem. The inclusion of BrC decreases OH by up to 30% over South America in September, up to 20% over southern Africa in July, and up to 15% over other biomass burning regions. Global annual mean OH concentrations in GEOS-Chem decrease due to the presence of absorbing BrC, increasing the methyl chloroform lifetime from 5.62 to 5.68 years, thus

Evaluating WRF-Chem multi-scale model in simulating aerosol radiative properties over the tropics – A case study over India

DOE Office of Scientific and Technical Information (OSTI.GOV)

Seethala, C.; Pandithurai, G.; Fast, Jerome D.

We utilized WRF-Chem multi-scale model to simulate the regional distribution of aerosols, optical properties and its effect on radiation over India for a winter month. The model is evaluated using measurements obtained from upper-air soundings, AERONET sun photometers, various satellite instruments, and pyranometers operated by the Indian Meteorological Department. The simulated downward shortwave flux was overestimated when the effect of aerosols on radiation and clouds was neglected. Downward shortwave radiation from a simulation that included aerosol-radiation interaction processes was 5 to 25 Wm{sup -2} closer to the observations, while a simulation that included aerosol-cloud interaction processes were another 1 tomore » 20 Wm{sup -2} closer to the observations. For the few observations available, the model usually underestimated particulate concentration. This is likely due to turbulent mixing, transport errors and the lack of secondary organic aerosol treatment in the model. The model efficiently captured the broad regional hotspots such as high aerosol optical depth over Indo-Gangetic basin as well as the northwestern and southern part of India. The regional distribution of aerosol optical depth compares well with AVHRR aerosol optical depth and the TOMS aerosol index. The magnitude and wavelength-dependence of simulated aerosol optical depth was also similar to the AERONET observations across India. Differences in surface shortwave radiation between simulations that included and neglected aerosol-radiation interactions were as high as -25 Wm{sup -2}, while differences in surface shortwave radiation between simulations that included and neglect aerosol-radiation-cloud interactions were as high as -30 Wm{sup -2}. The spatial variations of these differences were also compared with AVHRR observation. This study suggests that the model is able to qualitatively simulate the impact of aerosols on radiation over India; however, additional measurements of

Longwave Radiative Forcing of Saharan Dust Aerosols Estimated from MODIS, MISR and CERES Observations on Terra

NASA Technical Reports Server (NTRS)

Zhang, Jiang-Long; Christopher, Sundar A.

2003-01-01

Using observations from the Multi-angle Imaging Spectroradiometer (MISR), the Moderate Resolution Imaging Spectroradiometer (MODIS), and the Clouds and the Earth's Radiant Energy System (CERES) instruments onboard the Terra satellite; we present a new technique for studying longwave (LW) radiative forcing of dust aerosols over the Saharan desert for cloud-free conditions. The monthly-mean LW forcing for September 2000 is 7 W/sq m and the LW forcing efficiency' (LW(sub eff)) is 15 W/sq m. Using radiative transfer calculations, we also show that the vertical distribution of aerosols and water vapor are critical to the understanding of dust aerosol forcing. Using well calibrated, spatially and temporally collocated data sets, we have combined the strengths of three sensors from the same satellite to quantify the LW radiative forcing, and show that dust aerosols have a "warming" effect over the Saharan desert that will counteract the shortwave "cooling effect" of aerosols.

First observation-based estimates of cloud-free aerosol radiative forcing across China

Treesearch

Zhanqing Li; Kwon-Ho Lee; Yuesi Wang; Jinyuan Xin; Wei-Min Hao

2010-01-01

Heavy loading of aerosols in China is widely known, but little is known about their impact on regional radiation budgets, which is often expressed as aerosol radiative forcing (ARF). Cloud‐free direct ARF has either been estimated by models across the region or determined at a handful of locations with aerosol and/or radiation measurements. In this study, ARF...

Premonsoon Aerosol Characterization and Radiative Effects Over the Indo-Gangetic Plains: Implications for Regional Climate Warming

NASA Technical Reports Server (NTRS)

Gautam, Ritesh; Hsu, N. Christina; Lau, K.-M.

2010-01-01

The Himalayas have a profound effect on the South Asian climate and the regional hydrological cycle, as it forms a barrier for the strong monsoon winds and serves as an elevated heat source, thus controlling the onset and distribution of precipitation during the Indian summer monsoon. Recent studies have suggested that radiative heating by absorbing aerosols, such as dust and black carbon over the Indo-Gangetic Plains (IGP) and slopes of the Himalayas, may significantly accelerate the seasonal warming of the Hindu Kush-Himalayas-Tibetan Plateau (HKHT) and influence the subsequent evolution of the summer monsoon. This paper presents a detailed characterization of aerosols over the IGP and their radiative effects during the premonsoon season (April-May-June) when dust transport constitutes the bulk of the regional aerosol loading, using ground radiometric and spaceborne observations. During the dust-laden period, there is a strong response of surface shortwave flux to aerosol absorption indicated by the diurnally averaged forcing efficiency of -70 W/sq m per unit optical depth. The simulated aerosol single-scattering albedo, constrained by surface flux and aerosol measurements, is estimated to be 0.89+/- 0.01 (at approx.550 nm) with diurnal mean surface and top-of-atmosphere forcing values ranging from -11 to -79.8 W/sq m and +1.4 to +12 W/sq m, respectively, for the premonsoon period. The model-simulated solar heating rate profile peaks in the lower troposphere with enhanced heating penetrating into the middle troposphere (5-6 km), caused by vertically extended aerosols over the IGP with peak altitude of approx.5 km as indicated by spaceborne Cloud-Aerosol Lidar with Orthogonal Polarization observations. On a long-term climate scale, our analysis, on the basis of microwave satellite measurements of tropospheric temperatures from 1979 to 2007, indicates accelerated annual mean warming rates found over the Himalayan-Hindu Kush region (0.21 C/decade+/-0.08 C

Roles of production, consumption and trade in global and regional aerosol radiative forcing

NASA Astrophysics Data System (ADS)

Lin, J.; Tong, D.; Davis, S. J.; Ni, R.; Tan, X.; Pan, D.; Zhao, H.; Lu, Z.; Streets, D. G.; Feng, T.; Zhang, Q.; Yan, Y.; Hu, Y.; Li, J.; Liu, Z.; Jiang, X.; Geng, G.; He, K.; Huang, Y.; Guan, D.

2016-12-01

Anthropogenic aerosols exert strong radiative forcing on the climate system. Prevailing view regards aerosol radiative forcing as a result of emissions from regions' economic production, with China and other developing regions having the largest contributions to radiative forcing at present. However, economic production is driven by global demand for computation, and international trade allows for separation of regions consuming goods and services from regions where goods and related aerosol pollution are produced. It has recently been recognized that regions' consumption and trade have profoundly altered the spatial distribution of aerosol emissions and pollution. Building upon our previous work, this study quantifies for the first time the roles of trade and consumption in aerosol climate forcing attributed to different regions. We contrast the direct radiative forcing of aerosols related to regions' consumption of goods and services against the forcing due to emissions produced in each region. Aerosols assessed include black carbon, primary organic aerosol, and secondary inorganic aerosols including sulfate, nitrate and ammonium. We find that global aerosol radiative forcing due to emissions produced in East Asia is much stronger than the forcing related to goods and services ultimately consumed in that region because of its large net export of emissions-intensive goods. The opposite is true for net importers like Western Europe and North America: global radiative forcing related to consumption is much greater than the forcing due to emissions produced in these regions. Overall, trade is associated with a shift of radiative forcing from net importing to net exporting regions. Compared to greenhouse gases such as carbon dioxide, the short atmospheric lifetimes of aerosols cause large localized differences in radiative forcing. International efforts to reduce emissions in the exporting countries will help alleviate trade-related climate and health impacts of

Light Absorption Properties and Radiative Effects of Primary Organic Aerosol Emissions

EPA Science Inventory

Organic aerosols (OA) in the atmosphere affect Earth’s energy budget by not only scattering but also absorbing solar radiation due to the presence of the so-called “brown carbon” (BrC) component. However, the absorptivities of OA are not or poorly represented in current climate m...

Stratospheric aerosols and climatic change

NASA Technical Reports Server (NTRS)

Toon, O. B.; Pollack, J. B.

1978-01-01

Stratospht1ic sulfuric acid particles scatter and absorb sunlight and they scatter, absorb and emit terrestrial thermal radiation. These interactions play a role in the earth's radiation balance and therefore affect climate. The stratospheric aerosols are perturbed by volcanic injection of SO2 and ash, by aircraft injection of SO2, by rocket exhaust of Al2O3 and by tropospheric mixing of particles and pollutant SO2 and COS. In order to assess the effects of these perturbations on climate, the effects of the aerosols on the radiation balance must be understood and in order to understand the radiation effects the properties of the aerosols must be known. The discussion covers the aerosols' effect on the radiation balance. It is shown that the aerosol size distribution controls whether the aerosols will tend to warm or cool the earth's surface. Calculations of aerosol properties, including size distribution, for various perturbation sources are carried out on the basis of an aerosol model. Calculations are also presented of the climatic impact of perturbed aerosols due to volcanic eruptions and Space Shuttle flights.

Effect of Spectrally Varying Albedo of Vegetation Surfaces on Shortwave Radiation Fluxes and Aerosol Direct Radiative Forcing

NASA Technical Reports Server (NTRS)

Zhu, L.; Martins, J. V.; Yu, H.

2012-01-01

This study develops an algorithm for representing detailed spectral features of vegetation albedo based on Moderate Resolution Imaging Spectrometer (MODIS) observations at 7 discrete channels, referred to as the MODIS Enhanced Vegetation Albedo (MEVA) algorithm. The MEVA algorithm empirically fills spectral gaps around the vegetation red edge near 0.7 micrometers and vegetation water absorption features at 1.48 and 1.92 micrometers which cannot be adequately captured by the MODIS 7 channels. We then assess the effects of applying MEVA in comparison to four other traditional approaches to calculate solar fluxes and aerosol direct radiative forcing (DRF) at the top of atmosphere (TOA) based on the MODIS discrete reflectance bands. By comparing the DRF results obtained through the MEVA method with the results obtained through the other four traditional approaches, we show that filling the spectral gap of the MODIS measurements around 0.7 micrometers based on the general spectral behavior of healthy green vegetation leads to significant improvement in the instantaneous aerosol DRF at TOA (up to 3.02Wm(exp -2) difference or 48% fraction of the aerosol DRF, .6.28Wm(exp -2), calculated for high spectral resolution surface reflectance from 0.3 to 2.5 micrometers for deciduous vegetation surface). The corrections of the spectral gaps in the vegetation spectrum in the near infrared, again missed by the MODIS reflectances, also contributes to improving TOA DRF calculations but to a much lower extent (less than 0.27Wm(exp -2), or about 4% of the instantaneous DRF). Compared to traditional approaches, MEVA also improves the accuracy of the outgoing solar flux between 0.3 to 2.5 micrometers at TOA by over 60Wm(exp -2) (for aspen 3 surface) and aerosol DRF by over 10Wm(exp -2) (for dry grass). Specifically, for Amazon vegetation types, MEVA can improve the accuracy of daily averaged aerosol radiative forcing in the spectral range of 0.3 to 2.5 micrometers at equator at the

Spatially Refined Aerosol Direct Radiative Focusing Efficiencies

EPA Science Inventory

Global aerosol direct radiative forcing (DRF) is an important metric for assessing potential climate impacts of future emissions changes. However, the radiative consequences of emissions perturbations are not readily quantified nor well understood at the level of detail necessary...

Spatially Refined Aerosol Direct Radiative Forcing Efficiencies

EPA Science Inventory

Global aerosol direct radiative forcing (DRF) is an important metric for assessing potential climate impacts of future emissions changes. However, the radiative consequences of emissions perturbations are not readily quantified nor well understood at the level of detail necessary...

The effect of aerosols on northern hemisphere wintertime stationary waves

NASA Astrophysics Data System (ADS)

Lewinschal, Anna; Ekman, Annica M. L.

2010-05-01

Aerosol particles have a considerable impact on the energy budget of the atmosphere because of their ability to scatter and absorb incoming solar radiation. Since the beginning of the industrialisation a large increase has been seen mainly in the concentrations of sulphate and black carbon as a result of combustion of fossil fuel and biomass burning. Aerosol particles have a relatively short residence time in the atmosphere why the aerosol concentration shows a large variation spatially as well as in time where high concentrations are found close to emission sources. This leads to a highly varying radiative forcing pattern which modifies temperature gradients which in turn can alter the pressure distribution and lead to changes in the circulation in the atmosphere. In this study, the effect on the wintertime planetary scale waves on the northern hemisphere is specifically considered together with the regional climate impact due to changes in the stationary waves. To investigate the effect of aerosols on the circulation a global general circulation model based on the ECMWF operational forecast model is used (EC-Earth). The aerosol description in EC-Earth consists of prescribed monthly mean mass concentration fields of five different types of aerosols: sulphate, black carbon, organic carbon, dust and sea salt. Only the direct radiative effect is considered and the different aerosol types are treated as external mixtures. Changes in the stationary wave pattern are determined by comparing model simulations using present-day and pre-industrial concentrations of aerosol particles. Since the planetary scale waves largely influence the storm tracks and are an important part of the meridional heat transport, changes in the wave pattern may have substantial impact on the climate globally and locally. By looking at changes in the model simulations globally it can be found that the aerosol radiative forcing has the potential to change the stationary wave pattern. Furthermore

Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

DOE Office of Scientific and Technical Information (OSTI.GOV)

Feng, Y.; Kotamarthi, V. R.; Coulter, R.

Aerosol radiative effects and thermodynamic responses over South Asia are examined with the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of aerosol optical depths (AODs) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in northern India. The WRF-Chem model is found to heavily underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model's low bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profilesmore » averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day −1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond

MODIS Observation of Aerosols over Southern Africa During SAFARI 2000: Data, Validation, and Estimation of Aerosol Radiative Forcing

NASA Technical Reports Server (NTRS)

Ichoku, Charles; Kaufman, Yoram; Remer, Lorraine; Chu, D. Allen; Mattoo, Shana; Tanre, Didier; Levy, Robert; Li, Rong-Rong; Kleidman, Richard; Lau, William K. M. (Technical Monitor)

2001-01-01

Aerosol properties, including optical thickness and size parameters, are retrieved operationally from the MODIS sensor onboard the Terra satellite launched on 18 December 1999. The predominant aerosol type over the Southern African region is smoke, which is generated from biomass burning on land and transported over the southern Atlantic Ocean. The SAFARI-2000 period experienced smoke aerosol emissions from the regular biomass burning activities as well as from the prescribed burns administered on the auspices of the experiment. The MODIS Aerosol Science Team (MAST) formulates and implements strategies for the retrieval of aerosol products from MODIS, as well as for validating and analyzing them in order to estimate aerosol effects in the radiative forcing of climate as accurately as possible. These activities are carried out not only from a global perspective, but also with a focus on specific regions identified as having interesting characteristics, such as the biomass burning phenomenon in southern Africa and the associated smoke aerosol, particulate, and trace gas emissions. Indeed, the SAFARI-2000 aerosol measurements from the ground and from aircraft, along with MODIS, provide excellent data sources for a more intensive validation and a closer study of the aerosol characteristics over Southern Africa. The SAFARI-2000 ground-based measurements of aerosol optical thickness (AOT) from both the automatic Aerosol Robotic Network (AERONET) and handheld Sun photometers have been used to validate MODIS retrievals, based on a sophisticated spatio-temporal technique. The average global monthly distribution of aerosol from MODIS has been combined with other data to calculate the southern African aerosol daily averaged (24 hr) radiative forcing over the ocean for September 2000. It is estimated that on the average, for cloud free conditions over an area of 9 million square kin, this predominantly smoke aerosol exerts a forcing of -30 W/square m C lose to the terrestrial

Describing the direct and indirect radiative effects of atmospheric aerosols over Europe by using coupled meteorology-chemistry simulations: a contribution from the AQMEII-Phase II exercise

NASA Astrophysics Data System (ADS)

Jimenez-Guerrero, Pedro; Balzarini, Alessandra; Baró, Rocío; Curci, Gabriele; Forkel, Renate; Hirtl, Marcus; Honzak, Luka; Langer, Matthias; Pérez, Juan L.; Pirovano, Guido; San José, Roberto; Tuccella, Paolo; Werhahn, Johannes; Zabkar, Rahela

2014-05-01

The study of the response of the aerosol levels in the atmosphere to a changing climate and how this affects the radiative budget of the Earth (direct, semi-direct and indirect effects) is an essential topic to build confidence on climate science, since these feedbacks involve the largest uncertainties nowadays. Air quality-climate interactions (AQCI) are, therefore, a key, but uncertain contributor to the anthropogenic forcing that remains poorly understood. To build confidence in the AQCI studies, regional-scale integrated meteorology-atmospheric chemistry models (i.e., models with on-line chemistry) that include detailed treatment of aerosol life cycle and aerosol impacts on radiation (direct effects) and clouds (indirect effects) are in demand. In this context, the main objective of this contribution is the study and definition of the uncertainties in the climate-chemistry-aerosol-cloud-radiation system associated to the direct radiative forcing and the indirect effect caused by aerosols over Europe, using an ensemble of fully-coupled meteorology-chemistry model simulations with the WRF-Chem model run under the umbrella of AQMEII-Phase 2 international initiative. Simulations were performed for Europe for the entire year 2010. According to the common simulation strategy, the year was simulated as a sequence of 2-day time slices. For better comparability, the seven groups applied the same grid spacing of 23 km and shared common processing of initial and boundary conditions as well as anthropogenic and fire emissions. With exception of a simulation with different cloud microphysics, identical physics options were chosen while the chemistry options were varied. Two model set-ups will be considered here: one sub-ensemble of simulations not taking into account any aerosol feedbacks (the baseline case) and another sub-ensemble of simulations which differs from the former by the inclusion of aerosol-radiation feedback. The existing differences for meteorological

Relative Contributions of Regional and Sector Emissions to the Radiative Forcing of Aerosol-Radiation and Aerosol-Cloud Interactions Based on the AeroCOM Phase III/HTAP2 Experiment

NASA Astrophysics Data System (ADS)

Takemura, T.; Chin, M.

2014-12-01

It is important to understand relative contributions of each regional and sector emission of aerosols and their precursor gases to the regional and global mean radiative forcing of aerosol-radiation and aerosol-cloud interactions. This is because it is useful for international cooperation on controls of air pollution and anthropogenic climate change along most suitable reduction path of their emissions from each region and sector. The Task Force on Hemispheric Transport of Air Pollution (TF HTAP) under the United Nations researches the intercontinental transport of air pollutants including aerosols with strong support of the Aerosol Comparisons between Observations and Models (AeroCOM). The ongoing AeroCOM Phase III/HTAP2 experiment assesses relative contributions of regional and sector sources of aerosols and their precursor gases to the air quality using global aerosol transport models with latest emission inventories. In this study, the extended analyses on the relative contributions of each regional and sector emission to the radiative forcing of aerosol-radiation and aerosol-cloud interactions are done from the AeroCOM Phase III/HTAP2 experiment. Simulated results from MIROC-SPRINTARS and other some global aerosol models participating in the the AeroCOM Phase III/HTAP2 experiment are assessed. Acknowledgements: This study is based on the AeroCOM Phase III/HTAP2 experiment and partly supported by the Environment Research and Technology Development Fund (S-12-3) of the Ministry of the Environment, Japan.

Results of a comprehensive atmospheric aerosol-radiation experiment in the southwestern United States. I - Size distribution, extinction optical depth and vertical profiles of aerosols suspended in the atmosphere. II - Radiation flux measurements and

NASA Technical Reports Server (NTRS)

Deluisi, J. J.; Furukawa, F. M.; Gillette, D. A.; Schuster, B. G.; Charlson, R. J.; Porch, W. M.; Fegley, R. W.; Herman, B. M.; Rabinoff, R. A.; Twitty, J. T.

1976-01-01

Results are reported for a field test that was aimed at acquiring a sufficient set of measurements of aerosol properties required as input for radiative-transfer calculations relevant to the earth's radiation balance. These measurements include aerosol extinction and size distributions, vertical profiles of aerosols, and radiation fluxes. Physically consistent, vertically inhomogeneous models of the aerosol characteristics of a turbid atmosphere over a desert and an agricultural region are constructed by using direct and indirect sampling techniques. These results are applied for a theoretical interpretation of airborne radiation-flux measurements. The absorption term of the complex refractive index of aerosols is estimated, a regional variation in the refractive index is noted, and the magnitude of solar-radiation absorption by aerosols and atmospheric molecules is determined.

Influence of aerosols on surface reaching spectral irradiance and introduction to a new technique of estimating aerosol radiative forcing from high resolution spectral flux measurements

NASA Astrophysics Data System (ADS)

Rao, Roshan

2016-04-01

Aerosol radiative forcing estimates with high certainty are required in climate change studies. The approach in estimating the aerosol radiative forcing by using the chemical composition of aerosols is not effective as the chemical composition data with radiative properties are not widely available. We look into the approach where ground based spectral radiation flux measurement is made and along with an Radtiative transfer (RT) model, radiative forcing is estimated. Measurements of spectral flux were made using an ASD spectroradiometer with 350 - 1050 nm wavelength range and a 3nm resolution during around 54 clear-sky days during which AOD range was around 0.01 to 0.7. Simultaneous measurements of black carbon were also made using Aethalometer (Magee Scientific) which ranged from around 1.5 ug/m3 to 8 ug/m3. The primary study involved in understanding the sensitivity of spectral flux due to change in individual aerosol species (Optical properties of Aerosols and Clouds (OPAC) classified aerosol species) using the SBDART RT model. This made us clearly distinguish the influence of different aerosol species on the spectral flux. Following this, a new technique has been introduced to estimate an optically equivalent mixture of aerosol species for the given location. The new method involves matching different combinations of aerosol species in OPAC model and RT model as long as the combination which gives the minimum root mean squared deviation from measured spectral flux is obtained. Using the optically equivalent aerosol mixture and RT model, aerosol radiative forcing is estimated. Also an alternate method to estimate the spectral SSA is discussed. Here, the RT model, the observed spectral flux and spectral AOD is used. Spectral AOD is input to RT model and SSA is varied till the minimum root mean squared difference between observed and simulated spectral flux from RT model is obtained. The methods discussed are limited to clear sky scenes and its accuracy to derive

Long-term changes of aerosol optical and radiative properties and their role in global dimming and brightening

NASA Astrophysics Data System (ADS)

Hatzianastassiou, N.; Papadimas, C. D.; Matsoukas, C.; Pavlakis, K.; Fotiadi, A.; Wild, M.; Vardavas, I.

2009-04-01

Global dimming and brightening (GDB) have profound effects on the Earth's environment. For example, GDB counteracts or supplements greenhouse warming. Atmospheric aerosols, through their interaction with solar radiation (direct, indirect and semi-direct effects) can affect GDB. Changes in aerosol burden or other physical and optical properties can modify tendencies of GDB. For example, satellite observations of aerosol amounts, available since the early 1980s, but only over the oceans, indicate a downward trend since about 1990, consistent with the observed brightening during this period. There is a need, however, to investigate similar trends, but also over land, and to relate them with contemporary GDB. The seasonal and inter-annual variability of the natural, but also anthropogenic aerosol direct radiative effect on solar radiation at the Earth's surface (DREsurf) and the contribution of aerosols to global dimming and brightening (GDB) is estimated over the period 1984-2001. This is achieved by using a spectral radiative transfer model together with Total Ozone Mapping Spectrometer (TOMS) aerosol optical thickness (AOT) and other satellite (International Satellite Cloud Climatology Project, ISCCP-D2), NCEP/NCAR reanalysis and Global Aerosol Data Set (GADS) data for surface and atmospheric parameters. The major findings are mostly related to natural and less to anthropogenic aerosols because of limitations of the TOMS observational technique. The model results indicate that aerosols exert a strong surface cooling over the globe by reducing locally the incoming surface solar radiation by up to 70 W m-2. This direct radiative effect averaged over the globe for the period 1984-2001, is equivalent to 5 W m-2, associated with 6.5 and 3.5 W m-2, for the Northern and Southern Hemispheres, respectively. However, this aerosol DREsurf effect shows an important inter-annual variability as large as 200%. A strong solar brightening, or decreased aerosol DREsurf, by as much as

Radiative absorption enhancement from coatings on black carbon aerosols.

PubMed

Cui, Xinjuan; Wang, Xinfeng; Yang, Lingxiao; Chen, Bing; Chen, Jianmin; Andersson, August; Gustafsson, Örjan

2016-05-01

The radiative absorption enhancement of ambient black carbon (BC), by light-refractive coatings of atmospheric aerosols, constitutes a large uncertainty in estimates of climate forcing. The direct measurements of radiative absorption enhancement require the experimentally-removing the coating materials in ambient BC-containing aerosols, which remains a challenge. Here, the absorption enhancement of the BC core by non-absorbing aerosol coatings was quantified using a two-step removal of both inorganic and organic matter coatings of ambient aerosols. The mass absorption cross-section (MAC) of decoated/pure atmospheric BC aerosols of 4.4±0.8m(2)g(-1) was enhanced to 9.6±1.8m(2)g(-1) at 678-nm wavelength for ambiently-coated BC aerosols at a rural Northern China site. The enhancement of MAC (EMAC) rises from 1.4±0.3 in fresh combustion emissions to ~3 for aged ambient China aerosols. The three-week high-intensity campaign observed an average EMAC of 2.25±0.55, and sulfates were primary drivers of the enhanced BC absorption. Copyright © 2016 Elsevier B.V. All rights reserved.

Zonal Aerosol Direct and Indirect Radiative Forcing using Combined CALIOP, CERES, CloudSat, and CERES Data

NASA Astrophysics Data System (ADS)

Miller, W. F.; Kato, S.; Rose, F. G.; Sun-Mack, S.

2009-12-01

Under the NASA Energy and Water Cycle System (NEWS) program, cloud and aerosol properties derived from CALIPSO, CloudSat, and MODIS data then matched to the CERES footprint are used for irradiance profile computations. Irradiance profiles are included in the publicly available product, CCCM. In addition to the MODIS and CALIPSO generated aerosol, aerosol optical thickness is calculated over ocean by processing MODIS radiance through the Stowe-Ignatov algorithm. The CERES cloud mask and properties algorithm are use with MODIS radiance to provide additional cloud information to accompany the actively sensed data. The passively sensed data is the only input to the standard CERES radiative flux products. The combined information is used as input to the NASA Langley Fu-Liou radiative transfer model to determine vertical profiles and Top of Atmosphere shortwave and longwave flux for pristine, all-sky, and aerosol conditions for the special data product. In this study, the three sources of aerosol optical thickness will be compared directly and their influence on the calculated and measured TOA fluxes. Earlier studies indicate that the largest uncertainty in estimating direct aerosol forcing using aerosol optical thickness derived from passive sensors is caused by cloud contamination. With collocated CALIPSO data, we are able to estimate frequency of occurrence of cloud contamination, effect on the aerosol optical thickness and direct radiative effect estimates.

Aerosol Properties and Radiative Forcing over Kanpur during Severe Aerosol Loading Conditions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kaskaoutis, D. G.; Sinha, P. R.; Vinoj, V.

2013-11-01

Atmospheric aerosols over India exhibit large spatio-temporal fluctuation driven by the local monsoon system, emission rates and seasonally-changed air masses. The northern part of India is well-known for its high aerosol loading throughout the year due to anthropogenic emissions, dust influence and biomass burning. On certain circumstances and, under favorable weather conditions, the aerosol load can be severe, causing significant health concerns and climate implications. The present work analyzes the aerosol episode (AE) days and examines the modification in aerosol properties and radiative forcing during the period 2001-2010 based on Kanpur-AERONET sun photometer data. As AEs are considered the daysmore » having daily-mean aerosol optical depth (AOD) above the decadal mean + 1 STD (standard deviation); the threshold value is defined at 0.928. The results identify 277 out of 2095 days (13.2%) of AEs over Kanpur, which are most frequently observed during post-monsoon (78 cases, 18.6%) and monsoon (76, 14.7%) seasons due to biomass-burning episodes and dust influence, respectively. On the other hand, the AEs in winter and pre-monsoon are lower in both absolute and percentage values (65, 12.5% and 58, 9.1%, respectively). The modification in aerosol properties on the AE days is strongly related to season. Thus, in post-monsoon and winter the AEs are associated with enhanced presence of fine-mode aerosols and Black Carbon from anthropogenic pollution and any kind of burning, while in pre-monsoon and monsoon seasons they are mostly associated with transported dust. Aerosol radiative forcing (ARF) calculated using SBDART shows much more surface (~-69 to -97 Wm-2) and Top of Atmosphere cooling (-20 to -30 Wm-2) as well as atmospheric heating (~43 to 71 Wm-2) during the AE days compared to seasonal means. These forcing values are mainly controlled by the higher AODs and the modified aerosol characteristics (Angstrom α, SSA) during the AE days in each season and may

Trends in sulfate and organic aerosol mass in the Southeast U.S.: Impact on aerosol optical depth and radiative forcing

NASA Astrophysics Data System (ADS)

Attwood, A. R.; Washenfelder, R. A.; Brock, C. A.; Hu, W.; Baumann, K.; Campuzano-Jost, P.; Day, D. A.; Edgerton, E. S.; Murphy, D. M.; Palm, B. B.; McComiskey, A.; Wagner, N. L.; Sá, S. S.; Ortega, A.; Martin, S. T.; Jimenez, J. L.; Brown, S. S.

2014-11-01

Emissions of SO2 in the United States have declined since the early 1990s, resulting in a decrease in aerosol sulfate mass in the Southeastern U.S. of -4.5(±0.9)% yr-1 between 1992 and 2013. Organic aerosol mass, the other major aerosol component in the Southeastern U.S., has decreased more slowly despite concurrent emission reductions in anthropogenic precursors. Summertime measurements in rural Alabama quantify the change in aerosol light extinction as a function of aerosol composition and relative humidity. Application of this relationship to composition data from 2001 to 2013 shows that a -1.1(±0.7)% yr-1 decrease in extinction can be attributed to decreasing aerosol water mass caused by the change in aerosol sulfate/organic ratio. Calculated reductions in extinction agree with regional trends in ground-based and satellite-derived aerosol optical depth. The diurnally averaged summertime surface radiative effect has changed by 8.0 W m-2, with 19% attributed to the decrease in aerosol water.

Quantitative impact of aerosols on numerical weather prediction. Part I: Direct radiative forcing

NASA Astrophysics Data System (ADS)

Marquis, J. W.; Zhang, J.; Reid, J. S.; Benedetti, A.; Christensen, M.

2017-12-01

While the effects of aerosols on climate have been extensively studied over the past two decades, the impacts of aerosols on operational weather forecasts have not been carefully quantified. Despite this lack of quantification, aerosol plumes can impact weather forecasts directly by reducing surface reaching solar radiation and indirectly through affecting remotely sensed data that are used for weather forecasts. In part I of this study, the direct impact of smoke aerosol plumes on surface temperature forecasts are quantified using a smoke aerosol event affecting the United States Upper-Midwest in 2015. NCEP, ECMWF and UKMO model forecast surface temperature uncertainties are studied with respect to aerosol loading. Smoke aerosol direct cooling efficiencies are derived and the potential of including aerosol particles in operational forecasts is discussed, with the consideration of aerosol trends, especially over regions with heavy aerosol loading.

Aerosol effects on clouds and precipitation over the eastern China

NASA Astrophysics Data System (ADS)

Wang, W. C.; Chen, G.; Song, Y.

2017-12-01

Anthropogenic aerosols (sulfates, nitrates and black carbons) can act as cloud condensation nuclei to regulate cloud droplet number and size, thereby changing cloud radiative properties and atmospheric short- and long-wave radiation. These together with aerosol direct radiative effects in turn alter the circulation with likely effects on the spatial distribution of cloud and precipitation. We conduct WRF model simulations over the eastern China to investigate the aerosol-cloud-climate interactions. In general, more aerosols yield more but smaller cloud droplets and larger cloud water content, whereas the changes of vertical distribution of cloud cover exhibit strong regional variations. For example, the low-cloud fraction and water content increase by more than 10% over the west part of the Yangtze-Huai River Valley (YHRV) and the southeast coastal region, but decrease over the east part of the YHRV, and high-cloud fraction decreases in South and North China but increases in the YHRV. The radiative forcing of aerosols and cloud changes are compared, with focus on the effects of changes of vertical distribution of cloud properties (microphysics and fraction). The precipitation changes are found to be closely associated with the circulation change, which favors more (and longer duration) rainfall over the YHRV but less (and shorter) rainfall over other regions. Details of the circulation change and its associations with clouds and precipitation will be presented.

Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain

NASA Astrophysics Data System (ADS)

Ding, Jing; Zhang, Yufen; Han, Suqin; Xiao, Zhimei; Wang, Jiao; Feng, Yinchang

2018-05-01

Aerosol and water vapor radiative forcings, shortwave atmospheric heating rates and longwave atmospheric cooling rates were determined based on in situ physical and chemical measurements of aerosol, associated with the Mie theory and a radiative transfer model, LOWTRAN7, during the two haze episodes in the winter of 2013 in Tianjin, China. The aerosol types considered in LOWTRAN7 included rural, urban, marine, desert and custom aerosols. The default ratio of the absorption coefficient to the extinction coefficient for urban aerosol in LOWTRAN7 was approximately double of those found in this work, implying the weaker absorption ability of aerosols in the North China Plain (NCP). Moreover, the aerosol is assumed to be evenly distributed below 1 km of planetary boundary layer (PBL) on hazy days in LOWTRAN7. If the default urban aerosol optical properties and extinction profile in LOWTRAN7 is employed directly, a larger energy imbalance between the atmosphere and surface is generated and the warming effect of the aerosol is magnified. Hence, modified urban aerosol optical properties were established to replace the corresponding parameters' database in LOWTRAN7. The aerosol extinction profiles were obtained based on a 255-m meteorological tower and observed results from the studies about Tianjin. In the NCP, the aerosol had little impact on atmospheric counter radiation. The water vapor is the crucial factor that affects atmospheric counter radiation. Both modified high shortwave heating rates and longwave cooling rates occur near the surface due to the abundance of aerosol and water vapor. The modified net atmospheric heating rate near the surface is 1.2 K d-1 on hazy days and 0.3 K d-1 on non-hazy days. Compared with the default urban aerosol optical properties and its vertical distribution in LOWTRAN7, the feedback effect of the modified urban aerosol on the boundary layer may not necessarily result in a stable lower atmosphere, but depends on the aerosol light

Aerosol indirect effect on tropospheric ozone via lightning

NASA Astrophysics Data System (ADS)

Yuan, Tianle; Remer, Lorraine A.; Bian, Huisheng; Ziemke, Jerald R.; Albrecht, Rachel; Pickering, Kenneth E.; Oreopoulos, Lazaros; Goodman, Steven J.; Yu, Hongbin; Allen, Dale J.

2012-09-01

Tropospheric ozone (O3) is a pollutant and major greenhouse gas and its radiative forcing is still uncertain. Inadequate understanding of processes related to O3 production, in particular those natural ones such as lightning, contributes to this uncertainty. Here we demonstrate a new effect of aerosol particles on O3production by affecting lightning activity and lightning-generated NOx (LNOx). We find that lightning flash rate increases at a remarkable rate of 30 times or more per unit of aerosol optical depth. We provide observational evidence that indicates the observed increase in lightning activity is caused by the influx of aerosols from a volcano. Satellite data analyses show O3is increased as a result of aerosol-induced increase in lightning and LNOx, which is supported by modle simulations with prescribed lightning change. O3production increase from this aerosol-lightning-ozone link is concentrated in the upper troposphere, where O3 is most efficient as a greenhouse gas. In the face of anthropogenic aerosol increase our findings suggest that lightning activity, LNOx and O3, especially in the upper troposphere, have all increased substantially since preindustrial time due to the proposed aerosol-lightning-ozone link, which implies a stronger O3 historical radiative forcing. Aerosol forcing therefore has a warming component via its effect on O3 production and this component has mostly been ignored in previous studies of climate forcing related to O3and aerosols. Sensitivity simulations suggest that 4-8% increase of column tropospheric ozone, mainly in the tropics, is expected if aerosol-lighting-ozone link is parameterized, depending on the background emission scenario. We note, however, substantial uncertainties remain on the exact magnitude of aerosol effect on tropospheric O3 via lightning. The challenges for obtaining a quantitative global estimate of this effect are also discussed. Our results have significant implications for understanding past and

The Use of Remote Sensing to Resolve the Aerosol Radiative Forcing

NASA Technical Reports Server (NTRS)

Kaufman, Y. J.; Tanre, D.; Remer, Lorraine

1999-01-01

Satellites are used for remote sensing of aerosol optical thickness and optical properties in order to derive the aerosol direct and indirect radiative forcing of climate. Accuracy of the derived aerosol optical thickness is used as a measure of the accuracy in deriving the aerosol radiative forcing. Several questions can be asked to challenge this concept. Is the accuracy of the satellite-derived aerosol direct forcing limited to the accuracy of the measured optical thickness? What are the spectral bands needed to derive the total aerosol forcing? Does most of the direct or indirect aerosol forcing of climate originate from regions with aerosol concentrations that are high enough to be detected from space? What should be the synergism ground-based and space-borne remote sensing to solve the problem? We shall try to answer some of these questions, using AVIRIS airborne measurements and simulations.

Microphysical Cloud Regimes used as a tool to study Aerosol-Cloud-Precipitation-Radiation interactions

NASA Astrophysics Data System (ADS)

Cho, N.; Oreopoulos, L.; Lee, D.

2017-12-01

The presentation will examine whether the diagnostic relationships between aerosol and cloud-affected quantities (precipitation, radiation) obtained from sparse temporal resolution measurements from polar orbiting satellites can potentially demonstrate actual aerosol effects on clouds with appropriate analysis. The analysis relies exclusively on Level-3 (gridded) data and comprises systematic cloud classification in terms of "microphysical cloud regimes" (µCRs), aerosol optical depth (AOD) variations relative to a region's local seasonal climatology, and exploitation of the 3-hour difference between Terra (morning) and Aqua (afternoon) overpasses. Specifically, our presentation will assess whether Aerosol-Cloud-Precipitation-Radiation interactions (ACPRI) can be diagnosed by investigating: (a) The variations with AOD of afternoon cloud-affected quantities composited by afternoon or morning µCRs; (b) µCR transition diagrams composited by morning AOD quartiles; (c) whether clouds represented by ensemble cloud effective radius - cloud optical thickness joint histograms look distinct under low and high AOD conditions when preceded or followed by specific µCRs. We will explain how our approach addresses long-standing themes of the ACPRI problem such as the optimal ways to decompose the problem by cloud class, the prevalence and detectability of 1st/2nd aerosol indirect effects and invigoration, and the effectiveness of aerosol changes in inducing cloud modification at different segments of the AOD distribution.

The Impact of Atmospheric Aerosols on the Fraction of absorbed Photosynthetically Active Radiation

NASA Astrophysics Data System (ADS)

Veroustraete, Frank

2010-05-01

Aerosol pollution attracts a growing interest from atmospheric scientists with regard to their impact on health, the global climate and vegetation stress. A hypothesis, less investigated, is whether atmospheric aerosol interactions in the solar radiation field affect the amount of radiation absorbed by vegetation canopies and hence terrestrial vegetation productivity. Typically, aerosols affect vegetation canopy radiation absorption efficiency by altering the physical characteristics of solar radiation incoming on for example a forest canopy. It has been illustrated, that increasing mixing ratio's of atmospheric particulate matter lead to a higher fraction of diffuse sunlight as opposed to direct sunlight. It can be demonstrated, based on the application of atmospheric (MODTRAN) and leaf/canopy radiative transfer (LIBERTY/SPRINT) models, that radiation absorption efficiency in the PAR band of Picea like forests increases with increasing levels of diffuse radiation. It can be documented - on a theoretical basis - as well, that increasing aerosol loads in the atmosphere, induce and increased canopy PAR absorption efficiency. In this paper it is suggested, that atmospheric aerosols have to be taken into account when estimating vegetation gross primary productivity (GPP). The results suggest that Northern hemisphere vegetation CO2 uptake magnitude may increase with increasing atmospheric aerosol loads. Many climate impact scenario's related to vegetation productivity estimates, do not take this phenomenon into account. Boldly speaking, the results suggest a larger sink function for terrestrial vegetation than generally accepted. Keywords: Aerosols, vegetation, fAPAR, CO2 uptake, diffuse radiation.

Radiative Forcing Due to Major Aerosol Emitting Sectors in China and India

NASA Technical Reports Server (NTRS)

Streets, David G.; Shindell, Drew Todd; Lu, Zifeng; Faluvegi, Greg

2013-01-01

Understanding the radiative forcing caused by anthropogenic aerosol sources is essential for making effective emission control decisions to mitigate climate change. We examined the net direct plus indirect radiative forcing caused by carbonaceous aerosol and sulfur emissions in key sectors of China and India using the GISS-E2 chemistry-climate model. Diesel trucks and buses (67 mW/ sq. m) and residential biofuel combustion (52 mW/ sq. m) in India have the largest global mean, annual average forcings due mainly to the direct and indirect effects of BC. Emissions from these two sectors in China have near-zero net global forcings. Coal-fired power plants in both countries exert a negative forcing of about -30 mW/ sq. m from production of sulfate. Aerosol forcings are largest locally, with direct forcings due to residential biofuel combustion of 580 mW/ sq. m over India and 416 mW/ sq. m over China, but they extend as far as North America, Europe, and the Arctic

A Novel Method for Estimating Shortwave Direct Radiative Effect of Above-Cloud Aerosols Using CALIOP and MODIS Data

NASA Technical Reports Server (NTRS)

Zhang, Zhibo; Meyer, Kerry G.; Platnick, Steven; Oreopoulos, Lazaros; Lee, Dongmin; Yu, Hongbin

2014-01-01

This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It addresses the overlap of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure while also accounting for subgrid-scale variations of aerosols. The method is computationally efficient because of its use of grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table based on radiative transfer calculations. We verify that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous (approximately 1:30PM local time) shortwave DRE of above cloud aerosol (ACA) that generally agrees with more rigorous pixel-level computation within 4 percent. We also estimate the impact of potential CALIOP aerosol optical depth (AOD) retrieval bias of ACA on DRE. We find that the regional and seasonal mean instantaneous DRE of ACA over southeast Atlantic Ocean would increase, from the original value of 6.4 W m(-2) based on operational CALIOP AOD to 9.6 W m(-2) if CALIOP AOD retrieval are biased low by a factor of 1.5 (Meyer et al., 2013) and further to 30.9 W m(-2) if CALIOP AOD retrieval are biased low by a factor of 5 as suggested in (Jethva et al., 2014). In contrast, the instantaneous ACA radiative forcing efficiency (RFE) remains relatively invariant in all cases at about 53 W m(-2) AOD(-1), suggesting a near linear relation between the instantaneous RFE and AOD. We also compute the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global oceans based on 4 years of CALIOP and MODIS data. We find that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds. While we demonstrate our method using CALIOP and MODIS

Moderate Imaging Resolution Spectroradiometer (MODIS) Aerosol Optical Depth Retrieval for Aerosol Radiative Forcing

NASA Astrophysics Data System (ADS)

Asmat, A.; Jalal, K. A.; Ahmad, N.

2018-02-01

The present study uses the Aerosol Optical Depth (AOD) retrieved from Moderate Imaging Resolution Spectroradiometer (MODIS) data for the period from January 2011 until December 2015 over an urban area in Kuching, Sarawak. The results show the minimum AOD value retrieved from MODIS is -0.06 and the maximum value is 6.0. High aerosol loading with high AOD value observed during dry seasons and low AOD monitored during wet seasons. Multi plane regression technique used to retrieve AOD from MODIS (AODMODIS) and different statistics parameter is proposed by using relative absolute error for accuracy assessment in spatial and temporal averaging approach. The AODMODIS then compared with AOD derived from Aerosol Robotic Network (AERONET) Sunphotometer (AODAERONET) and the results shows high correlation coefficient (R2) for AODMODIS and AODAERONET with 0.93. AODMODIS used as an input parameters into Santa Barbara Discrete Ordinate Radiative Transfer (SBDART) model to estimate urban radiative forcing at Kuching. The observed hourly averaged for urban radiative forcing is -0.12 Wm-2 for top of atmosphere (TOA), -2.13 Wm-2 at the surface and 2.00 Wm-2 in the atmosphere. There is a moderate relationship observed between urban radiative forcing calculated using SBDART and AERONET which are 0.75 at the surface, 0.65 at TOA and 0.56 in atmosphere. Overall, variation in AOD tends to cause large bias in the estimated urban radiative forcing.

Global Radiative Forcing of Coupled Tropospheric Ozone and Aerosols in a Unified General Circulation Model

NASA Technical Reports Server (NTRS)

Liao, Hong; Seinfeld, John H.; Adams, Peter J.; Mickley, Loretta J.

2008-01-01

Global simulations of sea salt and mineral dust aerosols are integrated into a previously developed unified general circulation model (GCM), the Goddard Institute for Space Studies (GISS) GCM II', that simulates coupled tropospheric ozone-NOx-hydrocarbon chemistry and sulfate, nitrate, ammonium, black carbon, primary organic carbon, and secondary organic carbon aerosols. The fully coupled gas-aerosol unified GCM allows one to evaluate the extent to which global burdens, radiative forcing, and eventually climate feedbacks of ozone and aerosols are influenced by gas-aerosol chemical interactions. Estimated present-day global burdens of sea salt and mineral dust are 6.93 and 18.1 Tg with lifetimes of 0.4 and 3.9 days, respectively. The GCM is applied to estimate current top of atmosphere (TOA) and surface radiative forcing by tropospheric ozone and all natural and anthropogenic aerosol components. The global annual mean value of the radiative forcing by tropospheric ozone is estimated to be +0.53 W m(sup -2) at TOA and +0.07 W m(sup -2) at the Earth's surface. Global, annual average TOA and surface radiative forcing by all aerosols are estimated as -0.72 and -4.04 W m(sup -2), respectively. While the predicted highest aerosol cooling and heating at TOA are -10 and +12 W m(sup -2) respectively, surface forcing can reach values as high as -30 W m(sup -2), mainly caused by the absorption by black carbon, mineral dust, and OC. We also estimate the effects of chemistry-aerosol coupling on forcing estimates based on currently available understanding of heterogeneous reactions on aerosols. Through altering the burdens of sulfate, nitrate, and ozone, heterogeneous reactions are predicted to change the global mean TOA forcing of aerosols by 17% and influence global mean TOA forcing of tropospheric ozone by 15%.

Radiative transfer model for aerosols in infrared wavelengths for passive remote sensing applications.

PubMed

Ben-David, Avishai; Embury, Janon F; Davidson, Charles E

2006-09-10

A comprehensive analytical radiative transfer model for isothermal aerosols and vapors for passive infrared remote sensing applications (ground-based and airborne sensors) has been developed. The theoretical model illustrates the qualitative difference between an aerosol cloud and a chemical vapor cloud. The model is based on two and two/four stream approximations and includes thermal emission-absorption by the aerosols; scattering of diffused sky radiances incident from all sides on the aerosols (downwelling, upwelling, left, and right); and scattering of aerosol thermal emission. The model uses moderate resolution transmittance ambient atmospheric radiances as boundary conditions and provides analytical expressions for the information on the aerosol cloud that is contained in remote sensing measurements by using thermal contrasts between the aerosols and diffused sky radiances. Simulated measurements of a ground-based sensor viewing Bacillus subtilis var. niger bioaerosols and kaolin aerosols are given and discussed to illustrate the differences between a vapor-only model (i.e., only emission-absorption effects) and a complete model that adds aerosol scattering effects.

Case Studies of the Vertical Structure of the Direct Shortwave Aerosol Radiative Forcing During TARFOX

NASA Technical Reports Server (NTRS)

Redemann, J.; Turco, R. P.; Liou, K. N.; Hobbs, P. V.; Hartley, W. S.; Bergstrom, R. W.; Browell, E. V.; Russell, P. B.

2000-01-01

The vertical structure of aerosol-induced radiative flux changes in the Earth's troposphere affects local heating rates and thereby convective processes, the formation and lifetime of clouds, and hence the distribution of chemical constituents. We present observationally based estimates of the vertical structure of direct shortwave aerosol radiative forcing for two case studies from the Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) which took place on the U.S. east coast in July 1996. The aerosol radiative forcings are computed using the Fu-Liou broadband radiative transfer model. The aerosol optical properties used in the radiative transfer simulations are calculated from independent vertically resolved estimates of the complex aerosol indices of refraction in two to three distinct vertical layers, using profiles of in situ particle size distributions measured aboard the University of Washington research aircraft. Aerosol single-scattering albedos at 450 nm thus determined range from 0.9 to 0.985, while the asymmetry factor varies from 0.6 to 0.8. The instantaneous shortwave aerosol radiative forcings derived from the optical properties of the aerosols are of the order of -36 Wm(exp -2) at the top of the atmosphere and about -56 Wm(exp -2) at the surface for both case studies.

Top-of-Atmosphere Direct Radiative Effect of Aerosols from the Clouds and the Earth's Radiant Energy System Satellite Instrument (CERES)

NASA Technical Reports Server (NTRS)

Loeb, N. G.; Kato, S.

2002-01-01

Nine months of CERES/TRMM broadband fluxes combined with VIRS high-resolution imager measurements are used to estimate the daily average direct radiative effect of aerosols for clear-sky conditions over the tropical oceans. On average, aerosols have a cooling effect over the tropics of 4.6 +/- 1 W/sq m. The magnitude is approx.2 W/sq m smaller over the southern tropical oceans than it is over northern tropical oceans. The direct effect derived from CERES is highly correlated with coincident aerosol optical depth retrievals inferred from 0.63 microns VIRS radiances (correlation coefficient of 0.96). The slope of the regression line is approx. -32 W/sq m/t over the equatorial Pacific Ocean, but changes both regionally and seasonally, depending on the aerosol characteristics. Near sources of biomass burning and desert dust, the aerosol direct effect reaches -25 W sq m to -30 W/sq m. The direct effect from CERES also shows a dependence on wind speed. The reason for this dependence is unclear-it may be due to increased aerosol (e.g. sea-salt or aerosol transport) or increased surface reflection (e.g. due to whitecaps). The uncertainty in the tropical average direct effect from CERES is approx. 1 W/sq m (approx. 20%) due mainly to cloud contamination, the radiance-to-flux conversion, and instrument calibration. By comparison, uncertainties in the direct effect from the ERBE and CERES "ERBE-Like" products are a factor of 3 to 5 larger.

Impacts of ENSO events on cloud radiative effects in preindustrial conditions: Changes in cloud fraction and their dependence on interactive aerosol emissions and concentrations: IMPACT OF ENSO ON CLOUD RADIATIVE EFFECT

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yang, Yang; Russell, Lynn M.; Xu, Li

The impacts of the El Niño–Southern Oscillation (ENSO) events on shortwave and longwave cloud radiative effects (CRESW and CRELW) and the underlying changes in cloud fraction as well as aerosol emissions, wet scavenging and transport are quantified using three 150-year simulations in preindustrial conditions by the CESM model. Compared to recent observations from Clouds and the Earth’s Radiant Energy System (CERES), the model simulation successfully reproduced larger variations of CRESW over the tropical western and central Pacific, Indonesian regions, and the eastern Pacific Ocean, as well as large variations of CRELW located mainly within the tropics. The ENSO cycle ismore » found to dominate interannual variations of cloud radiative effects, especially over the tropics. Relative to those during La Niña events, simulated cooling (warming) effects from CRESW (CRELW) during El Niño events are stronger over the tropical western and central Pacific Ocean, with the largest difference exceeding 40 Wm–2 (30 Wm–2), with weaker effects of 10–30 Wm–2 over Indonesian regions and the subtropical Pacific Ocean. Sensitivity tests show that variations of cloud radiative effects are mainly driven by ENSO-related changes in cloud fraction. The variations in medium and high cloud fractions each account for about 20–50% of the interannual variations of CRESW over the tropics and almost all of the variations of CRELW between 60°S and 60°N. The variation of low cloud fraction contributes most interannual variations of CRESW over the mid-latitude oceans. Variations in natural aerosol concentrations considering emissions, wet scavenging and transport explained 10–30% of the interannual variations of both CRESW and CRELW over the tropical Pacific, Indonesian regions and the tropical Indian Ocean. Changes in wet scavenging of natural aerosol modulate the variations of cloud radiative effects. Because of increased (decreased) precipitation over the tropical western

Estimating the Direct Radiative Effect of Absorbing Aerosols Overlying Marine Boundary Layer Clouds in the Southeast Atlantic Using MODIS and CALIOP

NASA Technical Reports Server (NTRS)

Meyer, Kerry; Platnick, Steven; Oreopoulos, Lazaros; Lee, Dongmin

2013-01-01

Absorbing aerosols such as smoke strongly absorb solar radiation, particularly at ultraviolet and visible/near-infrared (VIS/NIR) wavelengths, and their presence above clouds can have considerable implications. It has been previously shown that they have a positive (i.e., warming) direct aerosol radiative effect (DARE) when overlying bright clouds. Additionally, they can cause biased passive instrument satellite retrievals in techniques that rely on VIS/NIR wavelengths for inferring the cloud optical thickness (COT) and effective radius (re) of underlying clouds, which can in turn yield biased above-cloud DARE estimates. Here we investigate Moderate Resolution Imaging Spectroradiometer (MODIS) cloud optical property retrieval biases due to overlying absorbing aerosols observed by Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and examine the impact of these biases on above-cloud DARE estimates. The investigation focuses on a region in the southeast Atlantic Ocean during August and September (2006-2011), where smoke from biomass burning in southern Africa overlies persistent marine boundary layer stratocumulus clouds. Adjusting for above-cloud aerosol attenuation yields increases in the regional mean liquid COT (averaged over all ocean-only liquid clouds) by roughly 6%; mean re increases by roughly 2.6%, almost exclusively due to the COT adjustment in the non-orthogonal retrieval space. It is found that these two biases lead to an underestimate of DARE. For liquid cloud Aqua MODIS pixels with CALIOP-observed above-cloud smoke, the regional mean above-cloud radiative forcing efficiency (DARE per unit aerosol optical depth (AOD)) at time of observation (near local noon for Aqua overpass) increases from 50.9Wm(sup-2)AOD(sup-1) to 65.1Wm(sup-2)AOD(sup -1) when using bias-adjusted instead of nonadjusted MODIS cloud retrievals.

Aerosol indirect effect on tropospheric ozone via lightning

NASA Astrophysics Data System (ADS)

Yuan, T.; Remer, L. A.; Bian, H.; Ziemke, J. R.; Albrecht, R. I.; Pickering, K. E.; Oreopoulos, L.; Goodman, S. J.; Yu, H.; Allen, D. J.

2012-12-01

Tropospheric ozone (O3) is a pollutant and major greenhouse gas and its radiative forcing is still uncertain. The unresolved difference between modeled and observed natural background O3 concentrations is a key source of the uncertainty. Here we demonstrate remarkable sensitivity of lightning activity to aerosol loading with lightning activity increasing more than 30 times per unit of aerosol optical depth over our study area. We provide observational evidence that indicates the observed increase in lightning activity is caused by the influx of aerosols from a volcano. Satellite data analyses suggest O3 is increased as a result of aerosol-induced increase in lightning and lightning produced NOx. Model simulations with prescribed lightning change corroborate the satellite data analysis. This aerosol-O3 connection is achieved via aerosol increasing lightning and thus lightning produced nitrogen oxides. This aerosol-lightning-ozone link provides a potential physical mechanism that may account for a part of the model-observation difference in background O3 concentration. More importantly, O3 production increase from this link is concentrated in the upper troposphere, where O3 is most efficient as a greenhouse gas. Both of these implications suggest a stronger O3 historical radiative forcing. This introduces a new pathway, through which increasing in aerosols from pre-industrial time to present day enhances tropospheric O3 production. Aerosol forcing thus has a warming component via its effect on O3 production. Sensitivity simulations suggest that 4-8% increase of tropospheric ozone, mainly in the tropics, is expected if aerosol-lighting-ozone link is parameterized, depending on the background emission scenario. We note, however, substantial uncertainties remain on the exact magnitude of aerosol effect on tropospheric O3 via lightning. The challenges for obtaining a quantitative global estimate of this effect are also discussed. Our results have significant implications

Radiative forcing by light-absorbing aerosols of pyrogenetic iron oxides.

PubMed

Ito, Akinori; Lin, Guangxing; Penner, Joyce E

2018-05-09

Iron (Fe) oxides in aerosols are known to absorb sun light and heat the atmosphere. However, the radiative forcing (RF) of light-absorbing aerosols of pyrogenetic Fe oxides is ignored in climate models. For the first time, we use a global chemical transport model and a radiative transfer model to estimate the RF by light-absorbing aerosols of pyrogenetic Fe oxides. The model results suggest that strongly absorbing Fe oxides (magnetite) contribute a RF that is about 10% of the RF due to black carbon (BC) over East Asia. The seasonal average of the RF due to dark Fe-rich mineral particles over East Asia (0.4-1.0 W m -2 ) is comparable to that over major biomass burning regions. This additional warming effect is amplified over polluted regions where the iron and steel industries have been recently developed. These findings may have important implications for the projection of the climate change, due to the rapid growth in energy consumption of the heavy industry in newly developing countries.

A study of 15-year aerosol optical thickness and direct shortwave aerosol radiative effect trends using MODIS, MISR, CALIOP and CERES

NASA Astrophysics Data System (ADS)

Alfaro-Contreras, Ricardo; Zhang, Jianglong; Reid, Jeffrey S.; Christopher, Sundar

2017-11-01

By combining Collection 6 Moderate Resolution and Imaging Spectroradiometer (MODIS) and Version 22 Multi-angle Imaging Spectroradiometer (MISR) aerosol products with Cloud and Earth's Radiant Energy System (CERES) flux products, the aerosol optical thickness (AOT, at 0.55 µm) and shortwave (SW) aerosol radiative effect (SWARE) trends are studied over ocean for the near-full Terra (2000-2015) and Aqua (2002-2015) data records. Despite differences in sampling methods, regional SWARE and AOT trends are highly correlated with one another. Over global oceans, weak SWARE (cloud-free SW flux) and AOT trends of 0.5-0.6 W m-2 (-0.5 to -0.6 W m-2) and 0.002 AOT decade-1 are found using Terra data. Near-zero AOT and SWARE trends are also found for using Aqua data, regardless of the angular distribution models (ADMs) used. Regionally, positive AOT and cloud-free SW flux (negative SWARE) trends are found over the Bay of Bengal, the Arabian Sea, the Arabian/Persian Gulf and the Red Sea, while statistically significant negative trends are derived over the Mediterranean Sea and the eastern US coast. In addition, the global mean instantaneous SW aerosol direct forcing efficiencies are found to be ˜ -60 W m-2 AOT-1, with corresponding SWARE values of ˜ -7 W m-2 from both Aqua and Terra data, again regardless of CERES ADMs used. Regionally, SW aerosol direct forcing efficiency values of ˜ -40 W m-2 AOT-1 are found over the southwest coast of Africa where smoke aerosol particles dominate in summer. Larger (in magnitude) SW aerosol direct forcing efficiency values of -50 to -80 W m-2 AOT-1 are found over several other dust- and pollutant-aerosol-dominated regions. Lastly, the AOT and SWARE trends from this study are also intercompared with aerosol trends (such as active-based ones) from several previous studies. Findings suggest that a cohesive understanding of the changing aerosol skies can be achieved through the analysis of observations from both passive- and active

Assessment of the Interactions Among Tropospheric Aerosol Loading, Radiative Balance and Clouds Through Examination of Their Multi-decadal Trends

EPA Science Inventory

While aerosol radiative effects have been recognized as some of the largest sources of uncertainty among the forcers of climate change, the verification of the spatial and temporal variability of aerosol radiative forcing has remained challenging. Anthropogenic emissions of prima...

Indirect aerosol effect increases CMIP5 models projected Arctic warming

DOE PAGES

Chylek, Petr; Vogelsang, Timothy J.; Klett, James D.; ...

2016-02-20

Phase 5 of the Coupled Model Intercomparison Project (CMIP5) climate models’ projections of the 2014–2100 Arctic warming under radiative forcing from representative concentration pathway 4.5 (RCP4.5) vary from 0.9° to 6.7°C. Climate models with or without a full indirect aerosol effect are both equally successful in reproducing the observed (1900–2014) Arctic warming and its trends. However, the 2014–2100 Arctic warming and the warming trends projected by models that include a full indirect aerosol effect (denoted here as AA models) are significantly higher (mean projected Arctic warming is about 1.5°C higher) than those projected by models without a full indirect aerosolmore » effect (denoted here as NAA models). The suggestion is that, within models including full indirect aerosol effects, those projecting stronger future changes are not necessarily distinguishable historically because any stronger past warming may have been partially offset by stronger historical aerosol cooling. In conclusion, the CMIP5 models that include a full indirect aerosol effect follow an inverse radiative forcing to equilibrium climate sensitivity relationship, while models without it do not.« less

Indirect aerosol effect increases CMIP5 models projected Arctic warming

DOE Office of Scientific and Technical Information (OSTI.GOV)

Chylek, Petr; Vogelsang, Timothy J.; Klett, James D.

Phase 5 of the Coupled Model Intercomparison Project (CMIP5) climate models’ projections of the 2014–2100 Arctic warming under radiative forcing from representative concentration pathway 4.5 (RCP4.5) vary from 0.9° to 6.7°C. Climate models with or without a full indirect aerosol effect are both equally successful in reproducing the observed (1900–2014) Arctic warming and its trends. However, the 2014–2100 Arctic warming and the warming trends projected by models that include a full indirect aerosol effect (denoted here as AA models) are significantly higher (mean projected Arctic warming is about 1.5°C higher) than those projected by models without a full indirect aerosolmore » effect (denoted here as NAA models). The suggestion is that, within models including full indirect aerosol effects, those projecting stronger future changes are not necessarily distinguishable historically because any stronger past warming may have been partially offset by stronger historical aerosol cooling. In conclusion, the CMIP5 models that include a full indirect aerosol effect follow an inverse radiative forcing to equilibrium climate sensitivity relationship, while models without it do not.« less

Monthly and seasonal variations of aerosol optical properties and direct radiative forcing over Zanjan, Iran

NASA Astrophysics Data System (ADS)

Gharibzadeh, Maryam; Alam, Khan; Abedini, Yousefali; Bidokhti, Abbasali Aliakbari; Masoumi, Amir

2017-11-01

Aerosol optical properties and radiative forcing over Zanjan in northwest of Iran has been analyzed during 2010-2013. The aerosol optical and radiative properties are less studied over Zanjan, and therefore, require a careful and in depth analysis. The optical properties like Aerosol Optical Depth (AOD), Ångström Exponent (AE), ASYmmetry parameter (ASY), Single Scattering Albedo (SSA), and Aerosol Volume Size Distribution (AVSD) have been evaluated using the ground-based AErosol RObotic NETwork (AERONET) data. Higher AOD while relatively lower AE were observed in the spring and summer, which showed the presence of coarse mode particles in these seasons. An obvious increase of coarse mode particles in AVSD distribution, as well as a higher value of SSA represented considerable addition of coarse mode particles like dust into the atmosphere of Zanjan in these two seasons. Increase in AE, while a decrease in AOD was detected in the winter and fall. The presence of fine particles indicates the dominance of particles like urban-industrial aerosols from local sources especially in the winter. The Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model was utilized to calculate the Aerosol Radiative Forcing (ARF) at the Top of the Atmosphere (TOA), earth's surface and within the atmosphere. The annual averaged ARF values were -13.47 W m-2 and -36.1 W m-2 at the TOA and earth's surface, respectively, which indicate a significant cooling effect. Likewise, the ARF efficiencies at the TOA and earth's surface were -65.08 W m-2 and -158.43 W m-2, respectively. The annual mean atmospheric ARF and heating rate within the atmosphere were 22.63 W m-2 and 0.27 Kday-1 respectively, represented the warming effect within the atmosphere. Finally, a good agreement was found between AERONET retrieved ARF and SBDART simulated ARF.

Contributions to the Understanding of Aerosol Microphysics Towards Improving the Assessment of Climate Radiative Forcing

NASA Astrophysics Data System (ADS)

Dawson, Kyle William

The study of climate and the associated impacts imposed by human activity has garnered the attention of scientists and policy makers since the 1950s. Research into the various atmospheric constituents that interact with solar radiation thus modulating Earth's radiative budget has been largely focused on the contributions from greenhouse gases and later focused on the role of atmospheric aerosol. The role of atmospheric aerosol, i.e. a solid or aqueous phase particulate, is complex and presents an opportunity for bettering the assessments of climate radiative forcing (i.e. the fraction of climate change due to anthropogenic, rather than natural, activities) in several ways. First, motivated to better understand the radiative effects of the Earth's background aerosol state to improve the assessment of anthropogenic effects, an experimental study on the water uptake ability of xanthan gum as a proxy for marine hydrogel, a component of natural primary emitted seaspray aerosol, is presented. Marine hydrogel comprises an organic component of the ocean surface microlayer that is released to the atmosphere via the bursting of bubbles generated by entrainment of air through crashing waves. This study investigates the water uptake ability (i.e. hygroscopicity) of these particles when exposed to a range of relative humidity (RH). The hydration characteristics of aerosolized pure xanthan gum as well as xanthan gum/salt mixtures were studied using a hygroscopic tandem differential mobility analyzer (HTDMA) and cloud condensation nuclei counter (CCNc). The hygroscopicity of the various solutions were compared to theoretical thermodynamic calculations accounting for the component volume fractions as a function of relative humidity. The data show that pure xanthan gum aerosol hygroscopicity behaves as other organic polysaccharides and, when combined with salts, is reasonably approximated by the volume fraction mixing rules above 90% RH. Deviations occur below 90% RH as well as for

Modeling the Relationships Between Aerosol Properties and the Direct and Indirect Effects of Aerosols on Climate

NASA Technical Reports Server (NTRS)

Toon, Owen B.

1994-01-01

Aerosols may affect climate directly by scattering and absorbing visible and infrared energy, They may also affect climate indirectly by modifying the properties of clouds through microphysical processes, and by altering abundances of radiatively important gases through heterogeneous chemistry. Researchers understand which aerosol properties control the direct effect of aerosols on the radiation budget. Unfortunately, despite an abundance of data on certain types of aerosols, much work remains to be done to determine the values of these properties. For instance we have little idea about the global distribution, seasonal variation, or interannual variability of the aerosol optical depth. Also we do not know the visible light absorption properties of tropical aerosols which may contain much debris from slash and burn agriculture. A positive correlation between aerosol concentrations and albedos of marine stratus clouds is observed, and the causative microphysics is understood. However, models suggest that it is difficult to produce new particles in the marine boundary layer. Some modelers have suggested that the particles in the marine boundary layer may originate in the free troposphere and be transported into the boundary layer. Others argue that the aerosols are created in the marine boundary layer. There are no data linking aerosol concentration and cirrus cloud albedo, and models suggest cirrus properties may not be very sensitive to aerosol abundance. There is clear evidence of a radiatively significant change in the global lower stratospheric ozone abundance during the past few decades. These changes are caused by heterogeneous chemical reactions occurring on the surfaces of particles. The rates of these reactions depend upon the chemical composition of the particles. Although rapid advances in understanding heterogeneous chemistry have been made, much remains to be done.

WRF-Chem simulations of aerosols and anthropogenic aerosol radiative forcing in East Asia

NASA Astrophysics Data System (ADS)

Gao, Yi; Zhao, Chun; Liu, Xiaohong; Zhang, Meigen; Leung, L. Ruby

2014-08-01

This study aims to provide a first comprehensive evaluation of WRF-Chem for modeling aerosols and anthropogenic aerosol radiative forcing (RF, including direct, semi-direct and indirect forcing) over East Asia. Several numerical experiments were conducted from November 2007 to December 2008. Comparison between model results and observations shows that the model can generally reproduce the observed spatial distributions of aerosol concentration, aerosol optical depth (AOD) and single scattering albedo (SSA) from measurements at many sites, including the relatively higher aerosol concentration and AOD over East China and the relatively lower AOD over Southeast Asia, Korea, and Japan. The model also depicts the seasonal variation and transport of pollutions over East Asia. Particulate matter of 10 μm or less in the aerodynamic diameter (PM10), black carbon (BC), sulfate (SO42-), nitrate (NO3-) and ammonium (NH4+) concentrations are higher in spring than other seasons in Japan, which indicates the possible influence of pollutant transport from polluted area of East Asia. The model underestimates SO42- and organic carbon (OC) concentrations over mainland China by about a factor of 2, while overestimates NO3- concentration in autumn along the Yangtze River. The model captures the dust events at the Zhangye site in the semi-arid region of China. AOD is high over Southwest and Central China in winter and spring and over North China in winter, spring and summer while is low over South China in summer due to monsoon precipitation. SSA is lowest in winter and highest in summer. Anthropogenic aerosol RF is estimated to range from -5 to -20 W m-2 over land and -20 to -40 W m-2 over adjacent oceans at the top of atmosphere (TOA), 5-30 W m-2 in the atmosphere (ATM) and -15 to -40 W m-2 at the bottom (BOT). The warming effect of anthropogenic aerosol in ATM results from BC aerosol while the negative aerosol RF at TOA is caused by scattering aerosols such as SO42-, NO3- and NH4

Optical, microphysical and radiative properties of aerosols over a tropical rural site in Kenya, East Africa: Source identification, modification and aerosol type discrimination

NASA Astrophysics Data System (ADS)

Boiyo, Richard; Kumar, K. Raghavendra; Zhao, Tianliang

2018-03-01

A better understanding of aerosol optical, microphysical and radiative properties is a crucial challenge for climate change studies. In the present study, column-integrated aerosol optical and radiative properties observed at a rural site, Mbita (0.42°S, 34.20 °E, and 1125 m above sea level) located in Kenya, East Africa (EA) are investigated using ground-based Aerosol Robotic Network (AERONET) data retrieved during January, 2007 to December, 2015. The annual mean aerosol optical depth (AOD500 nm), Ångström exponent (AE440-870 nm), fine mode fraction of AOD500 nm (FMF500 nm), and columnar water vapor (CWV, cm) were found to be 0.23 ± 0.08, 1.01 ± 0.16, 0.60 ± 0.07, and 2.72 ± 0.20, respectively. The aerosol optical properties exhibited a unimodal distribution with substantial seasonal heterogeneity in their peak values being low (high) during the local wet (dry) seasons. The observed data showed that Mbita and its environs are significantly influenced by various types of aerosols, with biomass burning and/or urban-industrial (BUI), mixed (MXD), and desert dust (DDT) aerosol types contributing to 37.72%, 32.81%, and 1.40%, respectively during the local dry season (JJA). The aerosol volume size distribution (VSD) exhibited bimodal lognormal structure with a geometric mean radius of 0.15 μm and 3.86-5.06 μm for fine- and coarse-mode aerosols, respectively. Further, analysis of single scattering albedo (SSA), asymmetry parameter (ASY) and refractive index (RI) revealed dominance of fine-mode absorbing aerosols during JJA. The averaged aerosol direct radiative forcing (ARF) retrieved from the AERONET showed a strong cooling effect at the bottom of the atmosphere (BOA) and significant warming within the atmosphere (ATM), representing the important role of aerosols played in this rural site of Kenya. Finally, the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model revealed that aerosols from distinct sources resulted in enhanced loading

Multi-site characterization of tropical aerosols: Implications for regional radiative forcing

NASA Astrophysics Data System (ADS)

Sumit, Kumar; Devara, P. C. S.; Manoj, M. G.

2012-03-01

A land campaign, as a part of the Indian Space Research Organization-Geosphere Biosphere Program (ISRO-GBP), has been organized using a suit of instruments like AERONET (Aerosol Robotic Network) Sun/Sky sunphotometer, Microtops-II (MICROprocessor-controlled Total Ozone Portable Spectrometer), short-wave pyranometer from December 1, 2006 to April 30, 2007, over five locations (Ahmedabad, Pune, Sinhgad, Trivandrum and Gadanki) representing different environments. The dominance of different aerosol types such as biomass burning, urban/industrial pollution, marine origin and desert-dust particles is expected at these five sites. In all locations, significant day-to-day variability in AOD and Ångström exponent is observed. The Ångström exponent exhibits its lowest values over semi-arid region (Ahmedabad) 0.4-0.7, while it is around 1.8 at rural site (Gadanki). The retrieved volume size distributions for Pune, Ahmedabad and Trivandrum are found to be bimodal with varying concentration of each mode. Interesting feature of this observation is, very low coarse-mode volume concentration observed at Trivandrum even though observations were made about 300 m from the coast. The synergy of results from these complementary measurements is reflected in the computed regional aerosol radiative forcing and heating rates. We have used a radiative transfer model (SBDART) to examine the variations of aerosol direct radiative effect (ADRE) and heating rates to give an overall estimation of the effect on climate. The ADRE, over different measurement sites, at short wavelength is found to be negative at the surface in the range of - 18 to - 59 W m - 2 , and TOA forcing values varied from + 0.9 to - 8 W m - 2 .

Sensitivity studies of different aerosol indirect effects in mixed-phase clouds

NASA Astrophysics Data System (ADS)

Lohmann, U.; Hoose, C.

2009-11-01

Aerosols affect the climate system by changing cloud characteristics. Using the global climate model ECHAM5-HAM, we investigate different aerosol effects on mixed-phase clouds: The glaciation effect, which refers to a more frequent glaciation due to anthropogenic aerosols, versus the de-activation effect, which suggests that ice nuclei become less effective because of an anthropogenic sulfate coating. The glaciation effect can partly offset the indirect aerosol effect on warm clouds and thus causes the total anthropogenic aerosol effect to be smaller. It is investigated by varying the parameterization for the Bergeron-Findeisen process and the threshold coating thickness of sulfate (SO4-crit), which is required to convert an externally mixed aerosol particle into an internally mixed particle. Differences in the net radiation at the top-of-the-atmosphere due to anthropogenic aerosols between the different sensitivity studies amount up to 0.5 W m-2. This suggests that the investigated mixed-phase processes have a major effect on the total anthropogenic aerosol effect.

Sensitivity studies of different aerosol indirect effects in mixed-phase clouds

NASA Astrophysics Data System (ADS)

Lohmann, U.; Hoose, C.

2009-07-01

Aerosols affect the climate system by changing cloud characteristics. Using the global climate model ECHAM5-HAM, we investigate different aerosol effects on mixed-phase clouds: The glaciation effect, which refers to a more frequent glaciation due to anthropogenic aerosols, versus the de-activation effect, which suggests that ice nuclei become less effective because of an anthropogenic sulfate coating. The glaciation effect can partly offset the indirect aerosol effect on warm clouds and thus causes the total anthropogenic aerosol effect to be smaller. It is investigated by varying the parameterization for the Bergeron-Findeisen process and the threshold coating thickness of sulfate (SO4-crit), which is required to convert an externally mixed aerosol particle into an internally mixed particle. Differences in the net radiation at the top-of-the-atmosphere due to anthropogenic aerosols between the different sensitivity studies amount up to 0.5 W m-2. This suggests that the investigated mixed-phase processes have a major effect on the total anthropogenic aerosol effect.