Science.gov

Sample records for area position-sensitive ionization

  1. A position-sensitive twin ionization chamber for fission fragment and prompt neutron correlation experiments

    NASA Astrophysics Data System (ADS)

    Göök, A.; Geerts, W.; Hambsch, F.-J.; Oberstedt, S.; Vidali, M.; Zeynalov, Sh.

    2016-09-01

    A twin position-sensitive Frisch grid ionization chamber, intended as a fission fragment detector in experiments to study prompt fission neutron correlations with fission fragment properties, is presented. Fission fragment mass and energies are determined by means of the double kinetic energy technique, based on conservation of mass and linear momentum. The position sensitivity is achieved by replacing each anode plate in the standard twin ionization chamber by a wire plane and a strip anode, both readout by means of resistive charge division. This provides information about the fission axis orientation, which is necessary to reconstruct the neutron emission process in the fully accelerated fragment rest-frame. The energy resolution compared to the standard twin ionization chamber is found not to be affected by the modification. The angular resolution of the detector relative to an arbitrarily oriented axis is better than 7° FWHM. Results on prompt fission neutron angular distributions in 235U(n,f) obtained with the detector in combination with an array of neutron scintillation detectors is presented as a proof of principle.

  2. Conformable large-area position-sensitive photodetectors based on luminescence-collecting silicone waveguides

    NASA Astrophysics Data System (ADS)

    Bartu, Petr; Koeppe, Robert; Arnold, Nikita; Neulinger, Anton; Fallon, Lisa; Bauer, Siegfried

    2010-06-01

    Position sensitive detection schemes based on the lateral photoeffect rely on inorganic semiconductors. Such position sensitive devices (PSDs) are reliable and robust, but preparation with large active areas is expensive and use on curved substrates is impossible. Here we present a novel route for the fabrication of conformable PSDs which allows easy preparation on large areas, and use on curved surfaces. Our device is based on stretchable silicone waveguides with embedded fluorescent dyes, used in conjunction with small silicon photodiodes. Impinging laser light (e.g., from a laser pointer) is absorbed by the dye in the PSD and re-emitted as fluorescence light at a larger wavelength. Due to the isotropic emission from the fluorescent dye molecules, most of the re-emitted light is coupled into the planar silicone waveguide and directed to the edges of the device. Here the light signals are detected via embedded small silicon photodiodes arranged in a regular pattern. Using a mathematical algorithm derived by extensive using of models from global positioning system (GPS) systems and human activity monitoring, the position of light spots is easily calculated. Additionally, the device shows high durability against mechanical stress, when clamped in an uniaxial stretcher and mechanically loaded up to 15% strain. The ease of fabrication, conformability, and durability of the device suggests its use as interface devices and as sensor skin for future robots.

  3. New beam line for time-of-flight medium energy ion scattering with large area position sensitive detector

    NASA Astrophysics Data System (ADS)

    Linnarsson, M. K.; Hallén, A.; Åström, J.; Primetzhofer, D.; Legendre, S.; Possnert, G.

    2012-09-01

    A new beam line for medium energy ion mass scattering (MEIS) has been designed and set up at the Ångström laboratory, Uppsala University, Sweden. This MEIS system is based on a time-of-flight (ToF) concept and the electronics for beam chopping relies on a 4 MHz function generator. Repetition rates can be varied between 1 MHz and 63 kHz and pulse widths below 1 ns are typically obtained by including beam bunching. A 6-axis goniometer is used at the target station. Scattering angle and energy of backscattered ions are extracted from a time-resolved and position-sensitive detector. Examples of the performance are given for three kinds of probing ions, 1H+, 4He+, and 11B+. Depth resolution is in the nanometer range and 1 and 2 nm thick Pt layers can easily be resolved. Mass resolution between nearby isotopes can be obtained as illustrated by Ga isotopes in GaAs. Taking advantage of the large size detector, a direct imaging (blocking pattern) of crystal channels are shown for hexagonal, 4H-SiC. The ToF-MEIS system described in this paper is intended for use in semiconductor and thin film areas. For example, depth profiling in the sub nanometer range for device development of contacts and dielectric interfaces. In addition to applied projects, fundamental studies of stopping cross sections in this medium energy range will also be conducted.

  4. Handy Compton camera using 3D position-sensitive scintillators coupled with large-area monolithic MPPC arrays

    NASA Astrophysics Data System (ADS)

    Kataoka, J.; Kishimoto, A.; Nishiyama, T.; Fujita, T.; Takeuchi, K.; Kato, T.; Nakamori, T.; Ohsuka, S.; Nakamura, S.; Hirayanagi, M.; Adachi, S.; Uchiyama, T.; Yamamoto, K.

    2013-12-01

    The release of radioactive isotopes (mainly 137Cs, 134Cs and 131I) from the crippled Fukushima Daiichi Nuclear Plant remains a serious problem in Japan. To help identify radiation hotspots and ensure effective decontamination operation, we are developing a novel Compton camera weighting only 1 kg and measuring just ∼10 cm2 in size. Despite its compactness, the camera realizes a wide 180° field of vision with a sensitivity about 50 times superior to other cameras being tested in Fukushima. We expect that a hotspot producing a 5 μSv/h dose at a distance of 3 m can be imaged every 10 s, with angular resolution better than 10° (FWHM). The 3D position-sensitive scintillators and thin monolithic MPPC arrays are the key technologies developed here. By measuring the pulse-height ratio of MPPC-arrays coupled at both ends of a Ce:GAGG scintillator block, the depth of interaction (DOI) is obtained for incident gamma rays as well as the usual 2D positions, with accuracy better than 2 mm. By using two identical 10 mm cubic Ce:GAGG scintillators as a scatterer and an absorber, we confirmed that the 3D configuration works well as a high-resolution gamma camera, and also works as spectrometer achieving typical energy resolution of 9.8% (FWHM) for 662 keV gamma rays. We present the current status of the prototype camera (weighting 1.5 kg and measuring 8.5×14×16 cm3 in size) being fabricated by Hamamatsu Photonics K.K. Although the camera still operates in non-DOI mode, angular resolution as high as 14° (FWHM) was achieved with an integration time of 30 s for the assumed hotspot described above.

  5. Position Sensitive Microcalorimeters

    NASA Technical Reports Server (NTRS)

    Sadleir, J. E.; Hammock, C.; Figueroa-Feliciano, E.; Stahle, C. K.; Bandler, S.; Saab, T.; Lindeman, M.; Porter, F. S.; Chervenak, J.; Brown, G.

    2004-01-01

    A Position Sensitive Transition-Edge Sensor (PoST) is a microcalorimeter device capable of one-dimensional imaging spectroscopy. The device consists of two Transition-Edge Sensors (TESs) connected to the ends of a long X-ray absorbing strip. The energy of a photon hitting the absorber and the position of the absorption event along the strip is measured from the response in the two sensors by analyzing the relative signal sizes, pulse rise times, and the sum of the pulses measured at each sensor, We report on the recent PoST effort at Goddard for applications to large field of view, high-energy- resolution, X-ray astrophysics.

  6. Development and applications of a new neutron single-crystal diffractometer based on a two-dimensional large-area curved position-sensitive detector

    PubMed Central

    Lee, Chang-Hee; Noda, Yukio; Ishikawa, Yoshihisa; Kim, Shin Ae; Moon, Myungkook; Kimura, Hiroyuki; Watanabe, Masashi; Dohi, Yuki

    2013-01-01

    A new single-crystal neutron diffractometer based on a large-area curved two-dimensional position-sensitive detector (C-2DPSD) has been developed. The diffractometer commissioning is almost complete, together with development of the measurement methodology and the raw data processing software package, the Reciprocal Analyzer, and the instrument is now ready to be launched for users. Position decoding of the C-2DPSD is via a delay-line readout method with an effective angular range of 110 × 54° in the horizontal and vertical directions, respectively, with a nominal radius of curvature of 530 mm. The diffractometer is equipped with a Ge(311) mosaic monochromator and two supermirror vacuum guide paths, one before and one after the monochromator position. The commissioning incorporates corrections and calibration of the instrument using an NaCl crystal, various applications such as crystallographic and magnetic structure measurements, a crystallinity check on large crystals, and a study on the composition or dopant content of a mixed crystal of (TmxYb1−x)Mn2O5. The installation of the diffractometer and the measurement method, the calibration procedure and results, the raw data treatment and visualization, and several applications using the large C-2DPSD-based diffractometer are reported. PMID:23682194

  7. Position-sensitive superconductor detectors

    NASA Astrophysics Data System (ADS)

    Kurakado, M.; Taniguchi, K.

    2016-12-01

    Superconducting tunnel junction (STJ) detectors and superconducting transition- edge sensors (TESs) are representative superconductor detectors having energy resolutions much higher than those of semiconductor detectors. STJ detectors are thin, thereby making it suitable for detecting low-energy X rays. The signals of STJ detectors are more than 100 times faster than those of TESs. By contrast, TESs are microcalorimeters that measure the radiation energy from the change in the temperature. Therefore, signals are slow and their time constants are typically several hundreds of μs. However, TESs possess excellent energy resolutions. For example, TESs have a resolution of 1.6 eV for 5.9-keV X rays. An array of STJs or TESs can be used as a pixel detector. Superconducting series-junction detectors (SSJDs) comprise multiple STJs and a single-crystal substrate that acts as a radiation absorber. SSJDs are also position sensitive, and their energy resolutions are higher than those of semiconductor detectors. In this paper, we give an overview of position-sensitive superconductor detectors.

  8. Position Sensitive Detection System for Charged Particles

    SciTech Connect

    Coello, E. A.; Favela, F.; Curiel, Q.; Chavez, E; Huerta, A.; Varela, A.; Shapira, Dan

    2012-01-01

    The position sensitive detection system presented in this work employs the Anger logic algorithm to determine the position of the light spark produced by the passage of charged particles on a 170 x 170 x 10 mm3 scintillator material (PILOT-U). The detection system consists of a matrix of nine photomultipliers, covering a fraction of the back area of the scintillators. Tests made with a non-collimated alpha particle source together with a Monte Carlo simulation that reproduces the data, suggest an intrinsic position resolution of up to 6 mm is achieved.

  9. A two-dimensional position sensitive gas chamber with scanned charge transfer readout

    NASA Astrophysics Data System (ADS)

    Gómez, F.; Iglesias, A.; Lobato, R.; Mosquera, J.; Pardo, J.; Pena, J.; Pazos, A.; Pombar, M.; Rodríguez, A.

    2003-10-01

    We have constructed and tested a two-dimensional position sensitive parallel-plate gas ionization chamber with scanned charge transfer readout. The scan readout method described here is based on the development of a new position-dependent charge transfer technique. It has been implemented by using gate strips perpendicularly oriented to the collector strips. This solution reduces considerably the number of electronic readout channels needed to cover large detector areas. The use of a 25 μm thick kapton etched circuit allows high charge transfer efficiency with a low gating voltage, consequently needing a very simple commutating circuit. The present prototype covers 8×8 cm2 with a pixel size of 1.27×1.27 mm2. Depending on the intended use and beam characteristics a smaller effective pixel is feasible and larger active areas are possible. This detector can be used for X-ray or other continuous beam intensity profile monitoring.

  10. Position Sensitive Proximity Charge Sensing Readout of HPGe Detectors

    NASA Astrophysics Data System (ADS)

    Priest, Anders Peterson

    Electrode segmentation is a necessity to achieve position sensitivity in semicon- ductor radiation detectors. Traditional segmentation requires decreasing electrode sizes while increasing channel numbers to achieve very fine position resolution. These electrodes can be complicated to fabricate, and many electrodes with individual electronic channels are required to instrument large detector areas. To simplify the fabrication process, we have moved the readout electrodes onto a printed circuit board that is positioned above the ionization type detection material. In this scheme, charge from radiation interactions will be shared amongst several electrodes, allowing for position interpolation. Because events can be reconstructed in between electrodes, fewer electrodes are needed to instrument large detector areas. The proximity charge sensing method of readout promises to simplify detector fabrication while maintaining the position resolution that is required by fields such as homeland security, astrophysics, environmental remediation, nuclear physics, and medical imaging. We performed scanning measurements on a proof of principle detector that we fabricated at Lawrence Berkeley National Laboratory (LBNL). These measurements showed that position resolution much finer than the strip pitch was achievable using the proximity charge readout method. We performed analytic calculations and Monte Carlo modeling to optimize the readout electrode geometry for a larger detector to test the limits of this technology. We achieved an average position resolution of 288 microm with eight proximity electrodes at a 5 mm pitch and 1 mm strip width, set 100 microm away from the detector surface by a Kapton spacer. To achieve this resolution using standard technologies, 300 microm pitch strips are necessary, and would require 100 channels to instrument the same area. Through our optimization calculations, we found that there is a trade-off between position resolution and energy resolution

  11. High speed curved position sensitive detector

    DOEpatents

    Hendricks, Robert W.; Wilson, Jack W.

    1989-01-01

    A high speed curved position sensitive porportional counter detector for use in x-ray diffraction, the detection of 5-20 keV photons and the like. The detector employs a planar anode assembly of a plurality of parallel metallic wires. This anode assembly is supported between two cathode planes, with at least one of these cathode planes having a serpentine resistive path in the form of a meander having legs generally perpendicular to the anode wires. This meander is produced by special microelectronic fabrication techniques whereby the meander "wire" fans outwardly at the cathode ends to produce the curved aspect of the detector, and the legs of the meander are small in cross-section and very closely spaced whereby a spatial resolution of about 50 .mu.m can be achieved. All of the other performance characteristics are about as good or better than conventional position sensitive proportional counter type detectors. Count rates of up to 40,000 counts per second with 0.5 .mu.s shaping time constants are achieved.

  12. An array of virtual Frisch-grid CdZnTe detectors and a front-end application-specific integrated circuit for large-area position-sensitive gamma-ray cameras

    SciTech Connect

    Bolotnikov, A. E.; Ackley, K.; Camarda, G. S.; Cherches, C.; Cui, Y.; De Geronimo, G.; Fried, J.; Hodges, D.; Hossain, A.; Lee, W.; Mahler, G.; Maritato, M.; Petryk, M.; Roy, U.; Salwen, C.; Vernon, E.; Yang, G.; James, R. B.

    2015-07-28

    We developed a robust and low-cost array of virtual Frisch-grid CdZnTe (CZT) detectors coupled to a front-end readout ASIC for spectroscopy and imaging of gamma rays. The array operates as a self-reliant detector module. It is comprised of 36 close-packed 6x6x15 mm3 detectors grouped into 3x3 sub-arrays of 2x2 detectors with the common cathodes. The front-end analog ASIC accommodates up to 36 anode and 9 cathode inputs. Several detector modules can be integrated into a single- or multi-layer unit operating as a Compton or a coded-aperture camera. We present the results from testing two fully assembled modules and readout electronics. The further enhancement of the arrays’ performance and reduction of their cost are made possible by using position-sensitive virtual Frisch-grid detectors, which allow for accurate corrections of the response of material non-uniformities caused by crystal defects.

  13. An array of virtual Frisch-grid CdZnTe detectors and a front-end application-specific integrated circuit for large-area position-sensitive gamma-ray cameras

    DOE PAGES

    Bolotnikov, A. E.; Ackley, K.; Camarda, G. S.; ...

    2015-07-28

    We developed a robust and low-cost array of virtual Frisch-grid CdZnTe (CZT) detectors coupled to a front-end readout ASIC for spectroscopy and imaging of gamma rays. The array operates as a self-reliant detector module. It is comprised of 36 close-packed 6x6x15 mm3 detectors grouped into 3x3 sub-arrays of 2x2 detectors with the common cathodes. The front-end analog ASIC accommodates up to 36 anode and 9 cathode inputs. Several detector modules can be integrated into a single- or multi-layer unit operating as a Compton or a coded-aperture camera. We present the results from testing two fully assembled modules and readout electronics.more » The further enhancement of the arrays’ performance and reduction of their cost are made possible by using position-sensitive virtual Frisch-grid detectors, which allow for accurate corrections of the response of material non-uniformities caused by crystal defects.« less

  14. An array of virtual Frisch-grid CdZnTe detectors and a front-end application-specific integrated circuit for large-area position-sensitive gamma-ray cameras.

    PubMed

    Bolotnikov, A E; Ackley, K; Camarda, G S; Cherches, C; Cui, Y; De Geronimo, G; Fried, J; Hodges, D; Hossain, A; Lee, W; Mahler, G; Maritato, M; Petryk, M; Roy, U; Salwen, C; Vernon, E; Yang, G; James, R B

    2015-07-01

    We developed a robust and low-cost array of virtual Frisch-grid CdZnTe detectors coupled to a front-end readout application-specific integrated circuit (ASIC) for spectroscopy and imaging of gamma rays. The array operates as a self-reliant detector module. It is comprised of 36 close-packed 6 × 6 × 15 mm(3) detectors grouped into 3 × 3 sub-arrays of 2 × 2 detectors with the common cathodes. The front-end analog ASIC accommodates up to 36 anode and 9 cathode inputs. Several detector modules can be integrated into a single- or multi-layer unit operating as a Compton or a coded-aperture camera. We present the results from testing two fully assembled modules and readout electronics. The further enhancement of the arrays' performance and reduction of their cost are possible by using position-sensitive virtual Frisch-grid detectors, which allow for accurate corrections of the response of material non-uniformities caused by crystal defects.

  15. An array of virtual Frisch-grid CdZnTe detectors and a front-end application-specific integrated circuit for large-area position-sensitive gamma-ray cameras

    SciTech Connect

    Bolotnikov, A. E. Ackley, K.; Camarda, G. S.; Cherches, C.; Cui, Y.; De Geronimo, G.; Fried, J.; Hossain, A.; Mahler, G.; Maritato, M.; Roy, U.; Salwen, C.; Vernon, E.; Yang, G.; James, R. B.; Hodges, D.; Lee, W.; Petryk, M.

    2015-07-15

    We developed a robust and low-cost array of virtual Frisch-grid CdZnTe detectors coupled to a front-end readout application-specific integrated circuit (ASIC) for spectroscopy and imaging of gamma rays. The array operates as a self-reliant detector module. It is comprised of 36 close-packed 6 × 6 × 15 mm{sup 3} detectors grouped into 3 × 3 sub-arrays of 2 × 2 detectors with the common cathodes. The front-end analog ASIC accommodates up to 36 anode and 9 cathode inputs. Several detector modules can be integrated into a single- or multi-layer unit operating as a Compton or a coded-aperture camera. We present the results from testing two fully assembled modules and readout electronics. The further enhancement of the arrays’ performance and reduction of their cost are possible by using position-sensitive virtual Frisch-grid detectors, which allow for accurate corrections of the response of material non-uniformities caused by crystal defects.

  16. Two-dimensional position sensitive radiation detectors

    DOEpatents

    Mihalczo, J.T.

    1994-02-22

    Nuclear reaction detectors capable of position sensitivity with submillimeter resolution in two dimensions are each provided by placing arrays of scintillation or wavelength shifting optical fibers formed of a plurality of such optical fibers in a side-by-side relationship in X and Y directions with a layer of nuclear reactive material operatively associated with surface regions of the optical fiber arrays. Each nuclear reaction occurring in the layer of nuclear reactive material produces energetic particles for simultaneously providing a light pulse in a single optical fiber in the X oriented array and in a single optical fiber in the Y oriented array. These pulses of light are transmitted to a signal producing circuit for providing signals indicative of the X-Y coordinates of each nuclear event. 6 figures.

  17. Two-dimensional position sensitive radiation detectors

    DOEpatents

    Mihalczo, John T.

    1994-01-01

    Nuclear reaction detectors capable of position sensitivity with submillimeter resolution in two dimensions are each provided by placing arrays of scintillation or wave length shifting optical fibers formed of a plurality of such optical fibers in a side-by-side relationship in X and Y directions with a layer of nuclear reactive material operatively associated with surface regions of the optical fiber arrays. Each nuclear reaction occurring in the layer of nuclear reactive material produces energetic particles for simultaneously providing a light pulse in a single optical fiber in the X oriented array and in a single optical fiber in the Y oriented array. These pulses of light are transmitted to a signal producing circuit for providing signals indicative of the X-Y coordinates of each nuclear event.

  18. Position-sensitive scanning fluorescence correlation spectroscopy.

    PubMed

    Skinner, Joseph P; Chen, Yan; Müller, Joachim D

    2005-08-01

    Fluorescence correlation spectroscopy (FCS) uses a stationary laser beam to illuminate a small sample volume and analyze the temporal behavior of the fluorescence fluctuations within the stationary observation volume. In contrast, scanning FCS (SFCS) collects the fluorescence signal from a moving observation volume by scanning the laser beam. The fluctuations now contain both temporal and spatial information about the sample. To access the spatial information we synchronize scanning and data acquisition. Synchronization allows us to evaluate correlations for every position along the scanned trajectory. We use a circular scan trajectory in this study. Because the scan radius is constant, the phase angle is sufficient to characterize the position of the beam. We introduce position-sensitive SFCS (PSFCS), where correlations are calculated as a function of lag time and phase. We present the theory of PSFCS and derive expressions for diffusion, diffusion in the presence of flow, and for immobilization. To test PSFCS we compare experimental data with theory. We determine the direction and speed of a flowing dye solution and the position of an immobilized particle. To demonstrate the feasibility of the technique for applications in living cells we present data of enhanced green fluorescent protein measured in the nucleus of COS cells.

  19. Position sensitivity of graphene field effect transistors to X-rays

    SciTech Connect

    Cazalas, Edward Moore, Michael E.; Jovanovic, Igor; Sarker, Biddut K.; Childres, Isaac; Chen, Yong P.

    2015-06-01

    Device architectures that incorporate graphene to realize detection of electromagnetic radiation typically utilize the direct absorbance of radiation by graphene. This limits their effective area to the size of the graphene and their applicability to lower-energy, less penetrating forms of radiation. In contrast, graphene-based transistor architectures that utilize the field effect as the detection mechanism can be sensitive to interactions of radiation not only with graphene but also with the surrounding substrate. Here, we report the study of the position sensitivity and response of a graphene-based field effect transistor (GFET) to penetrating, well-collimated radiation (micro-beam X-rays), producing ionization in the substrate primarily away from graphene. It is found that responsivity and response speed are strongly dependent on the X-ray beam distance from graphene and the gate voltage applied to the GFET. To develop an understanding of the spatially dependent response, a model is developed that incorporates the volumetric charge generation, transport, and recombination. The model is in good agreement with the observed spatial response characteristics of the GFET and predicts a greater response potential of the GFET to radiation interacting near its surface. The study undertaken provides the necessary insight into the volumetric nature of the GFET response, essential for development of GFET-based detectors for more penetrating forms of ionizing radiation.

  20. READOUT ASIC FOR 3D POSITION-SENSITIVE DETECTORS.

    SciTech Connect

    DE GERONIMO,G.; VERNON, E.; ACKLEY, K.; DRAGONE, A.; FRIED, J.; OCONNOR, P.; HE, Z.; HERMAN, C.; ZHANG, F.

    2007-10-27

    We describe an application specific integrated circuit (ASIC) for 3D position-sensitive detectors. It was optimized for pixelated CZT sensors, and it measures, corresponding to an ionizing event, the energy and timing of signals from 121 anodes and one cathode. Each channel provides low-noise charge amplification, high-order shaping, along with peak- and timing-detection. The cathode's timing can be measured in three different ways: the first is based on multiple thresholds on the charge amplifier's voltage output; the second uses the threshold crossing of a fast-shaped signal; and the third measures the peak amplitude and timing from a bipolar shaper. With its power of 2 mW per channel the ASIC measures, on a CZT sensor Connected and biased, charges up to 100 fC with an electronic resolution better than 200 e{sup -} rms. Our preliminary spectral measurements applying a simple cathode/mode ratio correction demonstrated a single-pixel resolution of 4.8 keV (0.72 %) at 662 keV, with the electronics and leakage current contributing in total with 2.1 keV.

  1. ASIC for High Rate 3D Position Sensitive Detectors

    SciTech Connect

    Vernon, E.; De Geronimo, G.; Ackley, K.; Fried, J.; He, Z.; Herman, C.; Zhang, F.

    2010-06-16

    We report on the development of an application specific integrated circuit (ASIC) for 3D position sensitive detectors (3D PSD). The ASIC is designed to operate with pixelated wide bandgap sensors like Cadmium-Zinc-Telluride (CZT), Mercuric Iodide (Hgl2) and Thallium Bromide (TIBr). It measures the amplitudes and timings associated with an ionizing event on 128 anodes, the anode grid, and the cathode. Each channel provides low-noise charge amplification, high-order shaping with peaking time adjustable from 250 ns to 12 {micro}s, gain adjustable to 20 mV/fC or 120 mV/fC (for a dynamic range of 3.2 MeV and 530 keV in CZT), amplitude discrimination with 5-bit trimming, and positive and negative peak and timing detections. The readout can be full or sparse, based on a flag and single- or multi-cycle token passing. All channels, triggered channels only, or triggered with neighbors can be read out thus increasing the rate capability of the system to more than 10 kcps. The ASIC dissipates 330 mW which corresponds to about 2.5 mW per channel.

  2. Position-sensitive CZT detector module

    NASA Astrophysics Data System (ADS)

    Matteson, James L.; Duttweiler, Fred; Huszar, George L.; Leblanc, Philippe C.; Skelton, Robert E.; Stephan, Edwin A.; Hink, Paul L.; Dowkontt, Paul F.; Slavis, Kimberly R.; Tumer, Tumay O.; Kravis, Scott D.

    1998-07-01

    Coded mask imagers for future high energy x-ray astronomy missions will require detector planes with areas of hundreds to thousands of cm(superscript 2) and position resolutions < 1 mm. Such detectors will enable coded mask imagers to discover and study thousands of high energy x-ray sources. The UCSD/WU/UCR/NOVA collaboration has been developing CZT detector systems with crossed-strip readout to meet these requirements. We report progress on a compact detector module with 41 cm(superscript 2) area and 0.5 mm spatial resolution. The design includes the bias network and ASIC readout electronics, and allows modules to be combined in large area arrays with very high live-area factors. Results from laboratory and balloon flight tests are presented.

  3. Practical Considerations for Optimizing Position Sensitivity in Arrays of Position-sensitive TES's

    NASA Technical Reports Server (NTRS)

    Smith, Stephen J.; Bandler, Simon R.; Figueroa-Feliciano, Encetali; Iyomoto, Naoko; Kelley, Richard L.; Kilbourne, Caroline A.; Porder, Frederick S.; Sadleir, John E.

    2007-01-01

    We are developing Position-Sensitive Transitions-Edge Sensors (PoST's) for future X-ray astronomy missions such as NASA's Constellation-X. The PoST consists of one or more Transitions Edge Sensors (TES's) thermally connected to a large X-ray absorber, which through heat diffusion, gives rise to position dependence. The development of PoST's is motivated by the desire to achieve the largest the focal-plan coverage with the fewest number of readout channels. In order to develop a practical array, consisting of an inner pixellated core with an outer array of large absorber PoST's, we must be able to simultaneously read out all (-1800) channels in the array. This is achievable using time division multiplexing (TDM), but does set stringent slew rate requirements on the array. Typically, we must damp the pulses to reduce the slew rate of the input signal to the TDM. This is achieved by applying a low-pass analog filter with large inductance to the signal. This attenuates the high frequency components of the signal, essential for position discrimination in PoST's, relative to the white noise of the readout chain and degrades the position sensitivity. Using numerically simulated data, we investigate the position sensing ability of typical PoST designs under such high inductance conditions. We investigate signal-processing techniques for optimal determination of the event position and discuss the practical considerations for real-time implementation.

  4. Practical Considerations for Optimizing Position Sensitivity in Arrays of Position-sensitive TES's

    NASA Technical Reports Server (NTRS)

    Smith, Stephen J.; Bandler, Simon R.; Figueroa-Feliciano, Encetali; Iyomoto, Naoko; Kelley, Richard L.; Kilbourne, Caroline A.; Porder, Frederick S.; Sadleir, John E.

    2007-01-01

    We are developing Position-Sensitive Transitions-Edge Sensors (PoST's) for future X-ray astronomy missions such as NASA's Constellation-X. The PoST consists of one or more Transitions Edge Sensors (TES's) thermally connected to a large X-ray absorber, which through heat diffusion, gives rise to position dependence. The development of PoST's is motivated by the desire to achieve the largest the focal-plan coverage with the fewest number of readout channels. In order to develop a practical array, consisting of an inner pixellated core with an outer array of large absorber PoST's, we must be able to simultaneously read out all (-1800) channels in the array. This is achievable using time division multiplexing (TDM), but does set stringent slew rate requirements on the array. Typically, we must damp the pulses to reduce the slew rate of the input signal to the TDM. This is achieved by applying a low-pass analog filter with large inductance to the signal. This attenuates the high frequency components of the signal, essential for position discrimination in PoST's, relative to the white noise of the readout chain and degrades the position sensitivity. Using numerically simulated data, we investigate the position sensing ability of typical PoST designs under such high inductance conditions. We investigate signal-processing techniques for optimal determination of the event position and discuss the practical considerations for real-time implementation.

  5. Emulation workbench for position sensitive gaseous scintillation detectors

    NASA Astrophysics Data System (ADS)

    Pereira, L.; Margato, L. M. S.; Morozov, A.; Solovov, V.; Fraga, F. A. F.

    2015-12-01

    Position sensitive detectors based on gaseous scintillation proportional counters with Anger-type readout are being used in several research areas such as neutron detection, search for dark matter and neutrinoless double beta decay. Design and optimization of such detectors are complex and time consuming tasks. Simulations, while being a powerful tool, strongly depend on the light transfer models and demand accurate knowledge of many parameters, which are often not available. Here we describe an alternative approach based on the experimental evaluation of a detector using an isotropic point-like light source with precisely controllable light emission properties, installed on a 3D positioning system. The results obtained with the developed setup at validation conditions, when the scattered light is strongly suppressed show good agreement with simulations.

  6. Position sensitive detector for fluorescence lifetime imaging

    NASA Astrophysics Data System (ADS)

    Prokazov, Y.; Turbin, E.; Weber, A.; Hartig, R.; Zuschratter, W.

    2014-12-01

    We present a detector system with a microchannel plate based photomultiplier tube (MCP-PMT) and its application for fluorescence lifetime imaging (FLIM) in visible light. A capacity coupled imaging technique (charge image) combined with a charge division anode is employed for the positional readout. Using an artificial neural network's (ANN) computation model we are able to reconstruct the position of the incident photon as precise as 20 microns over the detector active area of 25 mm diameter. Thus, the resulting image quality corresponds roughly to a megapixel conventional CCD camera. Importantly, it is feasible to reach such resolution using only 9 charge acquisition channels supporting the anode structure of 14 interconnected readout electrodes. Additionally, the system features better than 50 ps temporal resolution allowing single photon counting FLIM acquisition with a regular fluorescence wide-field microscope.

  7. 43 CFR 422.11 - Position sensitivity and investigations.

    Code of Federal Regulations, 2012 CFR

    2012-10-01

    ... 43 Public Lands: Interior 1 2012-10-01 2011-10-01 true Position sensitivity and investigations. 422.11 Section 422.11 Public Lands: Interior Regulations Relating to Public Lands BUREAU OF... Requirements § 422.11 Position sensitivity and investigations. Each law enforcement contract or cooperative...

  8. 43 CFR 422.11 - Position sensitivity and investigations.

    Code of Federal Regulations, 2014 CFR

    2014-10-01

    ... 43 Public Lands: Interior 1 2014-10-01 2014-10-01 false Position sensitivity and investigations. 422.11 Section 422.11 Public Lands: Interior Regulations Relating to Public Lands BUREAU OF... Requirements § 422.11 Position sensitivity and investigations. Each law enforcement contract or cooperative...

  9. 43 CFR 422.11 - Position sensitivity and investigations.

    Code of Federal Regulations, 2010 CFR

    2010-10-01

    ... 43 Public Lands: Interior 1 2010-10-01 2010-10-01 false Position sensitivity and investigations. 422.11 Section 422.11 Public Lands: Interior Regulations Relating to Public Lands BUREAU OF... Requirements § 422.11 Position sensitivity and investigations. Each law enforcement contract or cooperative...

  10. 43 CFR 422.11 - Position sensitivity and investigations.

    Code of Federal Regulations, 2013 CFR

    2013-10-01

    ... 43 Public Lands: Interior 1 2013-10-01 2013-10-01 false Position sensitivity and investigations. 422.11 Section 422.11 Public Lands: Interior Regulations Relating to Public Lands BUREAU OF... Requirements § 422.11 Position sensitivity and investigations. Each law enforcement contract or cooperative...

  11. 43 CFR 422.11 - Position sensitivity and investigations.

    Code of Federal Regulations, 2011 CFR

    2011-10-01

    ... 43 Public Lands: Interior 1 2011-10-01 2011-10-01 false Position sensitivity and investigations. 422.11 Section 422.11 Public Lands: Interior Regulations Relating to Public Lands BUREAU OF... Requirements § 422.11 Position sensitivity and investigations. Each law enforcement contract or cooperative...

  12. Dosimetric characterization of a large area pixel-segmented ionization chamber.

    PubMed

    Amerio, S; Boriano, A; Bourhaleb, F; Cirio, R; Donetti, M; Fidanzio, A; Garelli, E; Giordanengo, S; Madon, E; Marchetto, F; Nastasi, U; Peroni, C; Piermattei, A; Sanz Freire, C J; Sardo, A; Trevisiol, E

    2004-02-01

    A pixel-segmented ionization chamber has been designed and built by Torino University and INFN. The detector features a 24 x 24 cm2 active area divided in 1024 independent cylindrical ionization chambers and can be read out in 500 micros without introducing dead time; the digital charge quantum can be adjusted between 100 fC and 800 fC. The sensitive volume of each single ionization chamber is 0.07 cm3. The purpose of the detector is to ease the two-dimensional (2D) verifications of fields with complex shapes and large gradients. The detector was characterized in a PMMA phantom using 60Co and 6 MV x-ray photon beams. It has shown good signal linearity with respect to dose and dose rate to water. The average sensitivity of a single ionization chamber was 2.1 nC/Gy, constant within 0.5% over one month of daily measurements. Charge collection efficiency was 0.985 at the operating polarization voltage of 400 V and 3.5 Gy/min dose rate. Tissue maximum ratio and output factor have been compared with a Farmer ionization chamber and were found in good agreement. The dose profiles have been compared with the ones obtained with an ionization chamber in water phantom for the field sizes supplied by a 3D-Line dynamic multileaf collimator. These results show that this detector can be used for 2D dosimetry of x-ray photon beams, supplying a good spatial resolution and sensibly reducing the time spent in dosimetric verification of complex radiation fields.

  13. Theory and development of position-sensitive quantum calorimeters

    NASA Astrophysics Data System (ADS)

    Figueroa Feliciano, Enectali

    Quantum calorimeters are being developed as imaging spectrometers for future X-ray astrophysics observatories. Much of the science to be done by these instruments could benefit greatly from larger focal-plane coverage of the detector (without increasing pixel size). An order of magnitude more area will greatly increase the science throughput of these future instruments. One of the main deterrents to achieving this goal is the complexity of the readout schemes involved. We devised a way to increase the number of pixels from the current baseline designs by an order of magnitude without increasing the number of channels required for readout. The instrument is a high energy resolution, distributed-readout imaging spectrometer called a Position-Sensitive Transition-Edge Sensor (PoST). A PoST is a quantum calorimeter consisting of two Transition-Edge Sensors (TESs) on the ends of a long absorber to do one-dimensional imaging spectroscopy. Comparing rise time and energy information, the position of the event in the PoST is determined. Energy is inferred from the sum of the two pulses. We develop a generalized theoretical formalism for distributed-readout calorimeters and apply it to our devices. We derive the noise theory and calculate the theoretical energy resolution of a PoST. Our calculations show that a 7-pixel PoST with 6˜keV saturation energy can achieve 2.3˜eV resolution, making this a competitive design for future quantum calorimeter instruments. For this thesis we fabricated 7- and 15-pixel PoSTs using Mo/Au TESs and gold absorbers, and moved from concept drawings on scraps of napkins to a 32 eV at 1.5 keV energy resolution 7-pixel PoST calorimeter.

  14. Position sensitivity of MAMA detectors. [Multi-Anode Microchannel Array

    NASA Technical Reports Server (NTRS)

    Morgan, J. S.; Slater, D. S.; Timothy, J. G.; Jenkins, E. B.

    1988-01-01

    The results of laboratory and telescopic measurements of the position sensitivity of a visible MAMA detector utilizing a 'coarse-fine' array are presented. The photometric accuracy of this detector was determined under point source illumination. It was found that computed centroid positions are accurate across the entire array to within 0.04 pixels.

  15. Position sensitive radioactivity detection for gas and liquid chromatography

    DOEpatents

    Cochran, Joseph L.; McCarthy, John F.; Palumbo, Anthony V.; Phelps, Tommy J.

    2001-01-01

    A method and apparatus are provided for the position sensitive detection of radioactivity in a fluid stream, particularly in the effluent fluid stream from a gas or liquid chromatographic instrument. The invention represents a significant advance in efficiency and cost reduction compared with current efforts.

  16. Position sensitivity of MAMA detectors. [Multi-Anode Microchannel Array

    NASA Technical Reports Server (NTRS)

    Morgan, J. S.; Slater, D. S.; Timothy, J. G.; Jenkins, E. B.

    1988-01-01

    The results of laboratory and telescopic measurements of the position sensitivity of a visible MAMA detector utilizing a 'coarse-fine' array are presented. The photometric accuracy of this detector was determined under point source illumination. It was found that computed centroid positions are accurate across the entire array to within 0.04 pixels.

  17. Large-area field-ionization detector for the study of Rydberg atoms

    NASA Astrophysics Data System (ADS)

    Jones, A. C. L.; Piñeiro, A. M.; Roeder, E. E.; Rutbeck-Goldman, H. J.; Tom, H. W. K.; Mills, A. P.

    2016-11-01

    We describe here the development and characterization of a micro-channel plate (MCP) based detector designed for the efficient collection and detection of Rydberg positronium (Ps) atoms for use in a time-of-flight apparatus. The designed detector collects Rydberg atoms over a large area (˜4 times greater than the active area of the MCP), ionizing incident atoms and then collecting and focusing the freed positrons onto the MCP. Here we discuss the function, design, and optimization of the device. The detector has an efficiency for Rydberg Ps that is two times larger than that of the γ-ray scintillation detector based scheme it has been designed to replace, with half the background signal. In principle, detectors of the type described here could be readily employed for the detection of any Rydberg atom species, provided a sufficient field can be applied to achieve an ionization rate of ≥108/s. In such cases, the best time resolution would be achieved by collecting ionized electrons rather than the positive ions.

  18. Pharmaceutical cleaning validation using non-proximate large-area desorption electrospray ionization mass spectrometry.

    PubMed

    Soparawalla, Santosh; Salazar, Gary A; Perry, Richard H; Nicholas, Mark; Cooks, R Graham

    2009-01-01

    Desorption electrospray ionization (DESI) is a droplet-based ionization method that is applied to samples in the ambient environment with little or no sample preparation. Its utility for industrial applications is explored here for the case of pharmaceutical cleaning validation. A non-proximate large-area DESI system was built to examine representative areas of the surfaces of reaction vessels used in active product ingredient (API) manufacturing. A large-area sprayer capable of sampling an area of approximately 2.5 cm(2) was coupled with a transport tube to allow sensitive, representative sampling of APIs from a stainless steel surface 1 m away from the mass spectrometer. The system was used to detect the APIs neostigmine, acebutolol, amiloride, amiodarone, ibuprofen, montelukast, potassium clavulanate, and beta-estradiol, at levels as low as 30-10 ng/cm(2), easily satisfying the general acceptable limits set by the pharmaceutical industry. These levels were achieved from surfaces resembling the equipment used in API manufacturing processes at a rate of 30 s per analysis.

  19. Self-Balancing Position-Sensitive Detector (SBPSD).

    PubMed

    Porrazzo, Ryan; Lydecker, Leigh; Gattu, Suhasini; Bakhru, Hassaram; Tokranova, Natalya; Castracane, James

    2015-07-20

    Optical position-sensitive detectors (PSDs) are a non-contact method of tracking the location of a light spot. Silicon-based versions of such sensors are fabricated with standard CMOS technology, are inexpensive and provide a real-time, analog signal output corresponding to the position of the light spot. An innovative type of optical position sensor was developed using two back-to-back connected photodiodes. These so called self-balancing position-sensitive detectors (SBPSDs) eliminate the need for external readout circuitry entirely. Fabricated prototype devices demonstrate linear, symmetric coordinate characteristics and a spatial resolution of 200 μm for a 74 mm device. PSDs are commercially available only up to a length of 37 mm. Prototype devices were fabricated with various lengths up to 100 mm and can be scaled down to any size below that.

  20. Dual Position Sensitive MWPC for tracking reaction products at VAMOS++

    NASA Astrophysics Data System (ADS)

    Vandebrouck, M.; Lemasson, A.; Rejmund, M.; Fremont, G.; Pancin, J.; Navin, A.; Michelagnoli, C.; Goupil, J.; Spitaels, C.; Jacquot, B.

    2016-03-01

    The characteristics and performance of a Dual Position Sensitive Multi-Wire Proportional Counter (DPS-MWPC) used to measure the scattering angle, the interaction position on the target and the velocity of reaction products detected in the VAMOS++ magnetic spectrometer, are reported. The detector consists of a pair of position sensitive low pressure MWPCs and provides both fast timing signals, along with the two-dimensional position coordinates required to define the trajectory of the reaction products. A time-of-flight resolution of 305(11) ps (FWHM) was measured. The measured resolutions (FWHM) were 2.5(3) mrad and 560(70) μm for the scattering angle and the interaction point at the target respectively. The subsequent improvement of the Doppler correction of the energy of the γ-rays, detected in the γ-ray tracking array AGATA in coincidence with isotopically identified ions in VAMOS++, is also discussed.

  1. Development of a fast position-sensitive laser beam detector

    SciTech Connect

    Chavez, Isaac; Huang Rongxin; Henderson, Kevin; Florin, Ernst-Ludwig; Raizen, Mark G.

    2008-10-15

    We report the development of a fast position-sensitive laser beam detector. The detector uses a fiber-optic bundle that spatially splits the incident beam, followed by a fast balanced photodetector. The detector is applied to the study of Brownian motion of particles on fast time scales with 1 A spatial resolution. Future applications include the study of molecule motors, protein folding, as well as cellular processes.

  2. Quantitative analysis of molecular surfaces: areas, volumes, electrostatic potentials and average local ionization energies.

    PubMed

    Bulat, Felipe A; Toro-Labbé, Alejandro; Brinck, Tore; Murray, Jane S; Politzer, Peter

    2010-11-01

    We describe a procedure for performing quantitative analyses of fields f(r) on molecular surfaces, including statistical quantities and locating and evaluating their local extrema. Our approach avoids the need for explicit mathematical representation of the surface and can be implemented easily in existing graphical software, as it is based on the very popular representation of a surface as collection of polygons. We discuss applications involving the volumes, surface areas and molecular surface electrostatic potentials, and local ionization energies of a group of 11 molecules.

  3. A position sensitive microchannel photomultiplier for ultraviolet space astronomy

    NASA Technical Reports Server (NTRS)

    Lampton, M.; Siegmund, O. H. W.; Bixler, J.; Bowyer, S.

    1986-01-01

    The 25-mm microchannel-plate, position-sensitive UV astronomy photomultiplier tube presented is intended for the EOM-1 Spacelab Mission's FAUST payload and conducts wide-field imaging surveys in the VUV over the 1400-1800-A range. The sealed detector encompasses a CsI photocathode deposited on the inner surface of a MgF2 window, a stack of microchannel plates, and a wedge-and-strip two-dimensional position-sensing anode. Since the wedge-and-strip principle requires only three anode signals, flight electronics can be reduced to three charge amplifiers and three analog-to-digital converters.

  4. A position sensitive microchannel photomultiplier for ultraviolet space astronomy

    NASA Technical Reports Server (NTRS)

    Lampton, M.; Siegmund, O. H. W.; Bixler, J.; Bowyer, S.

    1986-01-01

    The 25-mm microchannel-plate, position-sensitive UV astronomy photomultiplier tube presented is intended for the EOM-1 Spacelab Mission's FAUST payload and conducts wide-field imaging surveys in the VUV over the 1400-1800-A range. The sealed detector encompasses a CsI photocathode deposited on the inner surface of a MgF2 window, a stack of microchannel plates, and a wedge-and-strip two-dimensional position-sensing anode. Since the wedge-and-strip principle requires only three anode signals, flight electronics can be reduced to three charge amplifiers and three analog-to-digital converters.

  5. A position sensitive phoswich hard X-ray detector system

    NASA Technical Reports Server (NTRS)

    Dean, A. J.; Hanson, C. G.; Hopkins, C. J.; Lewis, R. A.; Fraser-Mitchell, J.

    1985-01-01

    A prototype position sensitive phoswich hard X-ray detector, designed for eventual astronomical usage, was tested in the laboratory. The scintillation crystal geometry was designed on the basis of a Monte Carlo simulation of the internal optics and includes a 3mm thick NaI(T1) primary X-ray detector which is actively shielded by a 20 mm thick CsI(T1) scintillation crystal. This phoswich arrangement is viewed by a number two inch photomultipliers. Measured values of the positional and spectral resolution of incident X-ray photons are compared with calculation.

  6. Position-Sensitive Nuclear Spectroscopy with Pixel Detectors

    SciTech Connect

    Granja, Carlos; Vykydal, Zdenek; Jakubek, Jan; Pospisil, Stanislav

    2007-10-26

    State-of-the-art hybrid semiconductor pixel detectors such as Medipix2 are suitable for energy- and position-sensitive nuclear spectroscopy. In addition to excellent energy- and spatial-resolution, these devices can operate in spectroscopic, single-quantum counting and/or on-line tracking mode. A devoted compact USB-readout interface provides functionality and ease of operation. The compact and versatile Medipix2/USB radiation camera provides visualization, vacuum and room-temperature operation as a real-time portable active nuclear emulsion.

  7. Spectroscopy of Actinide Nuclei - Perspectives with Position Sensitive HPGe Detectors

    NASA Astrophysics Data System (ADS)

    Reiter, P.; Birkenbach, B.; Kotthaus, T.

    Recent advances in in-beam gamma-ray spectroscopy of actinide nuclei are based on highly efficient arrays of escape-suppressed spectrometers. The sensitivity of these detector arrays is greatly enhanced by the combination with powerful mass separators or particle detector systems. This technique is demonstrated by an experiment to investigate excited states in 234U after the one-neutron-transfer reaction 235U(d,t). In coincidence with the outgoing tritons, γ-rays were detected with the highly efficient MINIBALL spectrometer. In the near future an even enhanced sensitivity will be achieved by utilizing position sensitive HPGe detectors which will exploit the novel detection method of gamma-ray energy tracking in electrically segmented germanium detectors. An example for this novel approach is the investigation neutron-rich actinide Th and U nuclei after multi nucleon transfer reactions employing the AGATA demonstrator and PRISMA setup at LNL, Italy. A primary 136Xe beam hitting a 238U target was used to produce the nuclei of interest. Beam-like reaction products after neutron transfer were selected by the PRISMA spectrometer. Coincident γ-rays from excited states in beam and target like particles were measured with the position sensitive AGATA HPGe detectors. Improved Doppler correction and quality of the γ-spectra is based on the novel γ-ray tracking technique, which was successfully exploited in this region.

  8. Initial characterization of a position-sensitive photodiode/BGO detector for PET (positron emission tomography)

    SciTech Connect

    Derenzo, S.E.; Moses, W.W.; Jackson, H.G.; Turko, B.T.; Cahoon, J.L.; Geyer, A.B.; Vuletich, T.

    1988-11-01

    We present initial results of a position-sensitive photodiode/BGO detector for high resolution, multi-layer positron emission tomography (PET). Position sensitivity is achieved by dividing the 3 mm /times/ 20 mm rectangular photosensitive area along the diagonal to form two triangular segments. Each segment was individually connected to a low-noise amplifier. The photodiodes and crystals were cooled to /minus/100/degree/C to reduce dark current and increase the BGO signal. With an amplifier peaking time of 17 ..mu..sec, the sum of the signals (511 keV photopeak) was 3200 electrons with a full width at half maximum (fwhm) of 750 electrons. The ratio of one signal to the sum determined the depth of interaction with a resolution of 11 mm fwhm. 27 refs., 7 figs.

  9. Development of Three-Dimensional Position-Sensitive Room Temperature Semiconductor Gamma-Ray Spectrometers

    SciTech Connect

    Zhong He; Wen Li; Glenn F. Knoll; D. K. Wehe

    2000-06-04

    Semiconductor detectors can provide better spectroscopic performance than scintillation or gas-filled detectors because of the small ionization energy required to generate each electron-hole pair. Indeed, cryogenically cooled high-purity germanium detectors have played the dominant role whenever the best gamma-ray spectroscopy is required. A decades-long search for other semiconductor detectors that could provide higher stopping power and could operate at room temperature has been ongoing. Wide-bandgap semiconductors, such as CdTe, CdZnTe, and HgI{sub 2}, have captured the most attention. However, the use of these semiconductors in detectors has been hindered primarily by problems of charge trapping and material nonuniformity. Introduced in 1994, single-polarity charge sensing on semiconductor detectors has shown great promise in avoiding the hole-trapping problem, and the newly demonstrated three-dimensional position-sensing technique can significantly mitigate the degradation of energy resolution due to nonuniformity of detector material. In addition, three-dimensional position sensitivity will provide unique imaging capabilities of these gamma-ray spectrometers. These devices are of interest for nuclear nonproliferation, medical imaging, gamma-ray astronomy, and high-energy physics applications. This paper describes the three-dimensional position-sensing method and reports our latest results using second-generation three-dimensional position-sensitive semiconductor spectrometers.

  10. Particle tracking with scintillating fibers and position sensitive photomultipliers

    SciTech Connect

    C.F. Perdrisat; R. Pourang; D. Koechner; D. Raine, III; B. Kross; S. Majewski; A. Weisenberger; R. Wojcik; K. Zorn; V. Punjabi; A. Day

    1991-11-01

    The use of position-sensitive phototubes in conjunction with scintillating plastic fibers for a particle tracking application in a future focal plane polarimeter (FPP) in the hadron arm of the hall A HRS 2 facility at the Continuous Electron Beam Accelerator Facility (CEBAF). Current results indicate that the design parameters of the FPP in the hadron arm of the double spectrometer facility HRS2 can be met with a design which couples round or square fibers 3 mm in size to Hamamatsu R4135 phototubes. Position resolutions {sigma}x or {sigma}y on the order of 0.6 mm are obtained in the phototubes. Detector structures with staggered double fiber layers lead to overall resolution of {sigma}=1 mm, and detection efficiencies close to 1. The characteristic speed of these detectors makes them particularly appropriate for the high rates which are expected with the 200-{micro}A continuous wave beam at CEBAF.

  11. Functionalised hexagonal-domain graphene for position-sensitive photodetectors

    NASA Astrophysics Data System (ADS)

    De Sanctis, Adolfo; Barnes, Matthew D.; Amit, Iddo; Craciun, Monica F.; Russo, Saverio

    2017-03-01

    Graphene’s unique photoresponse has been largely used in a multitude of optoelectronics applications ranging from broadband photodetectors to wave-guide modulators. In this work we extend the range of applications to position-sensitive photodetectors (PSDs) using FeCl3-intercalated hexagonal domains of graphene grown by atmospheric pressure chemical vapour deposition (APCVD). The FeCl3-based chemical functionalisation of APCVD graphene crystals is affected by the presence of wrinkles and results in a non-uniform doping of the graphene layers. This doping profile creates multiple p-p+ photoactive junctions which show a linear and bipolar photoresponse with respect to the position of a focused light spot, which is ideal for the realization of a PSD. Our study paves the way towards the fabrication of flexible and transparent PSDs that could be embedded in smart textile and wearable electronics.

  12. Functionalised hexagonal-domain graphene for position-sensitive photodetectors.

    PubMed

    De Sanctis, Adolfo; Barnes, Matthew D; Amit, Iddo; Craciun, Monica F; Russo, Saverio

    2017-03-24

    Graphene's unique photoresponse has been largely used in a multitude of optoelectronics applications ranging from broadband photodetectors to wave-guide modulators. In this work we extend the range of applications to position-sensitive photodetectors (PSDs) using FeCl3-intercalated hexagonal domains of graphene grown by atmospheric pressure chemical vapour deposition (APCVD). The FeCl3-based chemical functionalisation of APCVD graphene crystals is affected by the presence of wrinkles and results in a non-uniform doping of the graphene layers. This doping profile creates multiple p-p(+) photoactive junctions which show a linear and bipolar photoresponse with respect to the position of a focused light spot, which is ideal for the realization of a PSD. Our study paves the way towards the fabrication of flexible and transparent PSDs that could be embedded in smart textile and wearable electronics.

  13. Silicon position sensitive detectors for the HELIOS (NA34) experiment

    SciTech Connect

    Beuttenmuller, R.; Bisi, V.; Chesi, E.; Di Nardo, R.P.; Esten, M.J.; Giubellino, P.; Kraner, H.W.; Ludlam, T.W.; Meddi, F.; Piuz, F.

    1986-03-01

    Silicon detectors having both ''pad'' and strip position sensitive configurations have been fabricated for the HELIOS experiment which requires an elaborate pulse height-dependent trigger as well as one dimensional silicon strip position sensing. The trigger detector is a 400 element, 30 mm diameter detector with readout connections from a ceramic overlay board. Tests with full prototype detectors have shown essentially 100% detection efficiency and excellent pulse height resolution well capable of delineating 0, 1 or 2 hits per pad. Strip detectors with 25 ..mu..m pitch and a varying readout pitch have been tested, which utilize both capacitive and resistive charge division. Techniques for realization of required interstrip resistors will be discussed and results which may compare these readout methods will be reported. 11 refs., 13 figs.

  14. A position-sensitive neutron spectrometer/dosimeter based on pressurized superheated drop (bubble) detectors

    NASA Astrophysics Data System (ADS)

    d'Errico, F.; Nath, R.; Holland, S. K.; Lamba, M.; Patz, S.; Rivard, M. J.

    2002-01-01

    A position-sensitive, superheated emulsion chamber (SEC) is introduced for three-dimensional (3D) spectrometry and dosimetry of fast neutrons. The detector is based on a fine suspension of octafluorocyclobutane droplets emulsified in a tissue-equivalent gel. This gel is highly viscous and immobilizes the bubbles at the location of their formation. At an operating temperature of 35°C, the droplets are moderately superheated and their evaporation is nucleated by the densely ionizing products of fast neutron interactions, with no response to sparsely ionizing radiations. Thus, when a neutron emitter such as a 252Cf brachytherapy source is inserted in the SEC, a bubble distribution forms around the source and makes the neutron field visible. The SEC is operated at different externally applied pressures that correspond to different response thresholds. These responses form a virtually orthogonal matrix which is suitable for spectrometry and allows the use of effective few channel unfolding procedures, yielding the spatial dependence of absorbed dose and neutron energy spectra in-tissue. Bubble spatial distributions in the chamber can be determined through optical tomography or magnetic resonance imaging (MRI). A 3D, steady-state MRI method has proven particularly effective for this purpose. After the imaging, the SEC can be pressurized above the halocarbon vapor tension in order to recondense the bubbles to the liquid phase. Within a few minutes, the device is annealed and ready to be used again for repeated measurements improving the bubble counting statistics.

  15. A New Positioning Algorithm for Position-Sensitive Avalanche Photodiodes

    PubMed Central

    Zhang, Jin; Olcott, Peter D.; Levin, Craig S.

    2013-01-01

    We are using a novel position sensitive avalanche photodiode (PSAPD) for the construction of a high resolution positron emission tomography (PET) camera. Up to now most researchers working with PSAPDs have been using an Anger-like positioning algorithm involving the four corner readout signals of the PSAPD. This algorithm yields a significant non-linear spatial “pin-cushion” distortion in raw crystal positioning histograms. In this paper, we report an improved positioning algorithm, which combines two diagonal corner signals of the PSAPD followed by a 45° rotation to determine the X or Y position of the interaction. We present flood positioning histogram data generated with the old and new positioning algorithms using a 3 × 4 array of 2 × 2 × 3 mm3 and a 3 × 8 array of 1 × 1 × 3 mm3 of LSO crystals coupled to 8 × 8 mm2 PSAPDs. This new algorithm significantly reduces the pin-cushion distortion in raw flood histogram image. PMID:24307743

  16. A New Positioning Algorithm for Position-Sensitive Avalanche Photodiodes.

    PubMed

    Zhang, Jin; Olcott, Peter D; Levin, Craig S

    2007-06-01

    We are using a novel position sensitive avalanche photodiode (PSAPD) for the construction of a high resolution positron emission tomography (PET) camera. Up to now most researchers working with PSAPDs have been using an Anger-like positioning algorithm involving the four corner readout signals of the PSAPD. This algorithm yields a significant non-linear spatial "pin-cushion" distortion in raw crystal positioning histograms. In this paper, we report an improved positioning algorithm, which combines two diagonal corner signals of the PSAPD followed by a 45° rotation to determine the X or Y position of the interaction. We present flood positioning histogram data generated with the old and new positioning algorithms using a 3 × 4 array of 2 × 2 × 3 mm(3) and a 3 × 8 array of 1 × 1 × 3 mm(3) of LSO crystals coupled to 8 × 8 mm(2) PSAPDs. This new algorithm significantly reduces the pin-cushion distortion in raw flood histogram image.

  17. Michrochannel plate for position sensitive alpha particle detection

    SciTech Connect

    Paul Hurley and James Tinsley

    2007-08-31

    This paper will describe the use of a microchannel plate (MCP) as the associated particle detector on a sealed tube neutron generator. The generator produces neutrons and associated alpha particles for use as a probe to locate and identify hidden explosives in associated particle imaging (API). The MCP measures the position in two dimensions and precise timing of the incident alpha particle, information which is then used to calculate the emission time and direction of the corresponding neutron. The MCP replaces the position-sensitive photomultipler tube (PSPMT) which, until recently, had been the only detector available for measuring position and timing for alpha particles in neutron generator applications. Where the PSPMT uses charge division for generating position information, a process that requires a first order correction to each pulse, the MCP uses delay-line timing, which requires no correction. The result is a device with an order of magnitude improvement in both position resolution and timing compared to the PSPMT. Hardware and software development and the measurements made to characterize the MCP for API applications are described.

  18. Canadian Penning Trap Mass Measurements using a Position Sensitive MCP

    NASA Astrophysics Data System (ADS)

    Kuta, Trenton; Aprahamian, Ani; Marley, Scott; Nystrom, Andrew; Clark, Jason; Perez Galvan, Adrian; Hirsh, Tsviki; Savard, Guy; Orford, Rodney; Morgan, Graeme

    2015-10-01

    The primary focus of the Canadian Penning Trap (CPT) located at Argonne National Lab is to determine the masses of various isotopes produced in the spontaneous fission of Californium. Currently, the CPT is operating in conjunction with CARIBU at the ATLAS facility in an attempt to measure neutron-rich nuclei produced by a 1.5 Curie source of Californium 252. The masses of nuclei produced in fission is accomplished by measuring the cyclotron frequency of the isotopes circling within the trap. This frequency is determined by a position sensitive MCP, which records the relative position of the isotope in the trap at different times. Using these position changes over time in connection with a center spot, angles between these positions are calculated and used to determine the frequency. Most of the work currently being conducted on the CPT is focused on the precision of these frequency measurements. The use of traps has revolutionized the measurements of nuclear masses to very high precision. The optimization methods employed here include focusing the beam in order to reduce the spread on the position of the isotope as well as the tuning of the MR-ToF, a mass separator that is intended on removing contaminants in the beam. This work was supported by the nuclear Grant PHY-1419765 for the University of Notre Dame.

  19. CdZnTe position-sensitive drift detectors with thicknesses up to 5 cm

    NASA Astrophysics Data System (ADS)

    Bolotnikov, A. E.; Camarda, G. S.; Chen, E.; Cheng, S.; Cui, Y.; Gul, R.; Gallagher, R.; Dedic, V.; De Geronimo, G.; Ocampo Giraldo, L.; Fried, J.; Hossain, A.; MacKenzie, J. M.; Sellin, P.; Taherion, S.; Vernon, E.; Yang, G.; El-hanany, U.; James, R. B.

    2016-02-01

    We investigated the feasibility of long-drift-time CdZnTe (CZT) gamma-ray detectors, fabricated from CZT material produced by Redlen Technologies. CZT crystals with cross-section areas of 5 × 5 mm2 and 6 × 6 mm2 and thicknesses of 20-, 30-, 40-, and 50-mm were configured as 3D position-sensitive drift detectors and were read out using a front-end ASIC. By correcting the electron charge losses caused by defects in the crystals, we demonstrated high performance for relatively thick detectors fabricated from unselected CZT material.

  20. Development of three-dimensional position-sensitive room temperature semiconductor gamma-ray spectrometers

    SciTech Connect

    He, Z.; Li, W.; Knoll, G.F.; Wehe, D.K.

    2000-07-01

    Semiconductor detectors can provide better spectroscopic performance than scintillation or gas-filled detectors because of the small ionization energy required to generate each electron-hole pair. Indeed, cryogenically cooled high-purity germanium detectors have played the dominant role whenever the best gamma-ray spectroscopy is required. A decades-long search for other semiconductor detectors that could provide higher stopping power and could operate at room temperature has been ongoing. Wide-band-gap semiconductors, such as CdTe, CdZnTe, and HgI{sub 2}, have captured the most attention. However, the use of these semiconductors in detectors has been hindered primarily by problems of charge trapping and material nonuniformity. Introduced in 1994, single-polarity charge sensing on semiconductor detectors has shown great promise in avoiding the hole-trapping problem, and the newly demonstrated three-dimensional position-sensing technique can significantly mitigate the degradation of energy resolution due to the nonuniformity of detector material. In addition, three-dimensional position sensitivity will provide unique imaging capabilities of these gamma-ray spectrometers. These devices are of interest for nuclear nonproliferation, medical imaging, gamma-ray astronomy, and high-energy physics applications. This paper reports the latest results using second-generation three-dimensional position-sensitive semiconductor spectrometers. The improvements over the first generation devices include: (1) Larger volume; (2) Improved anode design; (3) More reliable connections; (4) Enhanced electronic capability; and (5) Measurement of electron drift times. The new detectors and readout electronics (from IDE AS) are being assembled and tested.

  1. Signal and noise properties of position-sensitive avalanche photodiodes.

    PubMed

    Yang, Yongfeng; Wu, Yibao; Farrell, Richard; Dokhale, Purushottam A; Shah, Kanai S; Cherry, Simon R

    2011-10-07

    After many years of development, position-sensitive avalanche photodiodes (PSAPDs) are now being incorporated into a range of scintillation detector systems, including those used in high-resolution small-animal PET and PET/MR scanners. In this work, the signal, noise, signal-to-noise ratio (SNR), flood histogram and timing resolution were measured for lutetium oxyorthosilicate (LSO) scintillator arrays coupled to PSAPDs ranging in size from 10 to 20 mm, and the optimum bias voltage and working temperature were determined. Variations in the SNR performance of PSAPDs with the same dimensions were small, but the SNR decreased significantly with increasing PSAPD size and increasing temperature. Smaller PSAPDs (10 mm and 15 mm in width) produced acceptable flood histograms at 24 °C, and cooling lower than 16 °C produced little improvement. The optimum bias voltage was about 25 V below the break down voltage. The larger 20 mm PSAPDs have lower SNR and require cooling to 0-7 °C for acceptable performance. The optimum bias voltage is also lower (35 V or more below the break down voltage depending on the temperature). Significant changes in the timing resolution were observed as the bias voltage and temperature varied. Higher bias voltages provided better timing resolution. The best timing resolution obtained for individual crystals was 2.8 ns and 3.3 ns for the 10 mm and 15 mm PSAPDs, respectively. The results of this work provide useful guidance for selecting the bias voltage and working temperature for scintillation detectors that incorporate PSAPDs as the photodetector.

  2. Signal and Noise Properties of Position-Sensitive Avalanche Photodiodes

    PubMed Central

    Yang, Yongfeng; Wu, Yibao; Farrell, Richard; Dokhale, Purushottam A.; Shah, Kanai S.; Cherry, Simon R.

    2011-01-01

    After many years of development, position-sensitive avalanche photodiodes (PSAPDs) are now being incorporated into a range of scintillation detector systems, including those used in high-resolution small-animal PET and PET/MR scanners. In this work, the signal, noise, signal-to-noise ratio (SNR), flood histogram and timing resolution were measured for lutetium oxyorthosilicate (LSO) scintillator arrays coupled to PSAPDs ranging in size from 10–20 mm, and the optimum bias voltage and working temperature determined. Variations in the SNR performance of PSAPDs with the same dimensions were small, but the SNR decreased significantly with increasing PSAPD size and increasing temperature. Smaller PSAPDs (10 mm and 15 mm in width) produced acceptable flood histograms at 24 °C, and cooling lower than 16 °C produced little improvement. The optimum bias voltage was about 25 V below the break down voltage. The larger 20 mm PSAPDs have lower SNR and require cooling to 0–7 °C for acceptable performance. The optimum bias voltage also is lower (35 V or more below the break down voltage depending on the temperature). Significant changes in the timing resolution were observed as the bias voltage and temperature were varied. Higher bias voltages provided better timing resolution. The best timing resolution obtained for individual crystals was 2.8 ns and 3.3 ns for the 10 mm and 15 mm PSAPDs, respectively. The results of this work provide useful guidance for selecting the bias voltage and working temperature for scintillation detectors that incorporate PSAPDs as the photodetector. PMID:21896961

  3. Delay-Line Three-Dimensional Position Sensitive Radiation Detection

    NASA Astrophysics Data System (ADS)

    Jeong, Manhee

    High-resistivity silicon(Si) in large volumes and with good charge carrier transport properties has been produced and achieved success as a radiation detector material over the past few years due to its relatively low cost as well as the availability of well-established processing technologies. One application of that technology is in the fabrication of various position-sensing topologies from which the incident radiation's direction can be determined. We have succeeded in developing the modeling tools for investigating different position-sensing schemes and used those tools to examine both amplitude-based and time-based methods, an assessment that indicates that fine position-sensing can be achieved with simpler readout designs than are conventionally deployed. This realization can make ubiquitous and inexpensive deployment of special nuclear materials (SNM) detecting technology becomes more feasible because if one can deploy position-sensitive semiconductor detectors with only one or two contacts per side. For this purpose, we have described the delay-line radiation detector and its optimized fabrication. The semiconductor physics were simulated, the results from which guided the fabrication of the guard ring structure and the detector electrode, both of which included metal-field-plates. The measured improvement in the leakage current was confirmed with the fabricated devices, and the structures successfully suppressed soft-breakdown. We also demonstrated that fabricating an asymmetric strip-line structure successfully minimizing the pulse shaping and increases the distance through which one can propagate the information of the deposited charge distribution. With fabricated delay-line detectors we can acquire alpha spectra (Am-241) and gamma spectra (Ba-133, Co-57 and Cd-109). The delay-line detectors can therefore be used to extract the charge information from both ion and gamma-ray interactions. Furthermore, standard charge-sensitive circuits yield high SNR

  4. A systems approach to evaluating ionizing radiation: six focus areas to improve quality, efficiency, and patient safety.

    PubMed

    Perlin, Jonathan B; Mower, Laura; Bushe, Chris

    2015-01-01

    Ionizing radiation is an essential component of the care process. However, providers and patients may not be fully aware of the risks involved, the level of ionizing radiation delivered with various procedures, or the potential for harm through incidental overexposure or cumulative dose. Recent high-profile incidents demonstrating the devastating short-term consequences of radiation overexposure have drawn attention to these risks, but applicable solutions are lacking. Although various recommendations and guidelines have been proposed, organizational variability challenges providers to identify their own practical solutions. To identify potential failure modes and develop solutions to preserve patient safety within a large, national healthcare system, we assembled a multidisciplinary team to conduct a comprehensive analysis of practices surrounding the delivery of ionizing radiation. Workgroups were developed to analyze existing culture, processes, and technology to identify deficiencies and propose solutions. Six focus areas were identified: competency and certification; equipment; monitoring and auditing; education; clinical pathways; and communication and marketing. This manuscript summarizes this comprehensive, multidisciplinary, and systemic analysis of risk and provides examples to illustrate how these focus areas can be used to improve the use of ionizing radiation. The proposed solutions, once fully implemented, may advance patient safety and care.

  5. Development of Position-sensitive Transition-edge Sensor X-ray Detectors

    NASA Technical Reports Server (NTRS)

    Smith, S. J.; Bandler, S. R.; Brekosky, R. P.; Brown, A.-D.; Chervenak, J. A.; Eckard, M. E.; Finkbeiner, F. M.; Kelley, R. L.; Kilbourne, C. A.; Porter, F. s.; hide

    2008-01-01

    We report on the development of position-sensitive transition-edge sensors (PoST's) for future x-ray astronomy missions such as the International X-ray Observatory (IXO), currently under study by NASA and ESA. PoST's consist of multiple absorbers each with a different thermal coupling to one or more transition-edge sensor (TES). This differential thermal coupling between absorbers and TES's results in different characteristic pulse shapes and allows position discrimination between the different pixels. The development of PoST's is motivated by a desire to achieve maximum focal-plane area with the least number of readout channels and as such. PoST's are ideally suited to provide a focal-plane extension to the Constellation-X microcalorimeter array. We report the first experimental results of our latest one and two channel PoST's, which utilize fast thermalizing electroplated Au/Bi absorbers coupled to low noise Mo/Au TES's - a technology already successfully implemented in our arrays of single pixel TES's. We demonstrate 6 eV energy resolution coupled with spatial sensitivity in the keV energy range. We also report on the development of signal processing algorithms to optimize energy and position sensitivity of our detectors.

  6. Development of Position-sensitive Transition-edge Sensor X-ray Detectors

    NASA Technical Reports Server (NTRS)

    Smith, S. J.; Bandler, S. R.; Brekosky, R. P.; Brown, A.-D.; Chervenak, J. A.; Eckard, M. E.; Finkbeiner, F. M.; Kelley, R. L.; Kilbourne, C. A.; Porter, F. s.; Sad (eor. K/ E/); Figueroa-Feliciano, E.

    2008-01-01

    We report on the development of position-sensitive transition-edge sensors (PoST's) for future x-ray astronomy missions such as the International X-ray Observatory (IXO), currently under study by NASA and ESA. PoST's consist of multiple absorbers each with a different thermal coupling to one or more transition-edge sensor (TES). This differential thermal coupling between absorbers and TES's results in different characteristic pulse shapes and allows position discrimination between the different pixels. The development of PoST's is motivated by a desire to achieve maximum focal-plane area with the least number of readout channels and as such. PoST's are ideally suited to provide a focal-plane extension to the Constellation-X microcalorimeter array. We report the first experimental results of our latest one and two channel PoST's, which utilize fast thermalizing electroplated Au/Bi absorbers coupled to low noise Mo/Au TES's - a technology already successfully implemented in our arrays of single pixel TES's. We demonstrate 6 eV energy resolution coupled with spatial sensitivity in the keV energy range. We also report on the development of signal processing algorithms to optimize energy and position sensitivity of our detectors.

  7. Development of position-sensitive time-of-flight spectrometer for fission fragment research

    SciTech Connect

    Arnold, C. W.; Tovesson, F.; Meierbachtol, K.; Bredeweg, T.; Jandel, M.; Jorgenson, H. J.; Laptev, A.; Rusev, G.; Shields, D. W.; White, M.; Blakeley, R. E.; Mader, D. M.; Hecht, A. A.

    2014-07-09

    A position-sensitive, high-resolution time-of-flight detector for fission fragments has been developed. The SPectrometer for Ion DEtermination in fission Research (SPIDER) is a 2E–2v spectrometer designed to measure the mass of light fission fragments to a single mass unit. The time pick-off detector pairs to be used in SPIDER have been tested with α-particles from 229Th and its decay chain and α-particles and spontaneous fission fragments from 252Cf. Each detector module is comprised of thin electron conversion foil, electrostatic mirror, microchannel plates, and delay-line anodes. Particle trajectories on the order of 700 mm are determined accurately to within 0.7 mm. Flight times were measured with 250 ps resolution FWHM. Computed particle velocities are accurate to within 0.06 mm/ns corresponding to a precision of 0.5%. As a result, an ionization chamber capable of 400 keV energy resolution coupled with the velocity measurements described here will pave the way for modestly efficient measurements of light fission fragments with unit mass resolution.

  8. Development of position-sensitive time-of-flight spectrometer for fission fragment research

    DOE PAGES

    Arnold, C. W.; Tovesson, F.; Meierbachtol, K.; ...

    2014-07-09

    A position-sensitive, high-resolution time-of-flight detector for fission fragments has been developed. The SPectrometer for Ion DEtermination in fission Research (SPIDER) is a 2E–2v spectrometer designed to measure the mass of light fission fragments to a single mass unit. The time pick-off detector pairs to be used in SPIDER have been tested with α-particles from 229Th and its decay chain and α-particles and spontaneous fission fragments from 252Cf. Each detector module is comprised of thin electron conversion foil, electrostatic mirror, microchannel plates, and delay-line anodes. Particle trajectories on the order of 700 mm are determined accurately to within 0.7 mm. Flightmore » times were measured with 250 ps resolution FWHM. Computed particle velocities are accurate to within 0.06 mm/ns corresponding to a precision of 0.5%. As a result, an ionization chamber capable of 400 keV energy resolution coupled with the velocity measurements described here will pave the way for modestly efficient measurements of light fission fragments with unit mass resolution.« less

  9. Position-sensitive proportional counter with low-resistance metal-wire anode

    DOEpatents

    Kopp, Manfred K.

    1980-01-01

    A position-sensitive proportional counter circuit is provided which allows the use of a conventional (low-resistance, metal-wire anode) proportional counter for spatial resolution of an ionizing event along the anode of the counter. A pair of specially designed active-capacitance preamplifiers are used to terminate the anode ends wherein the anode is treated as an RC line. The preamplifiers act as stabilized active capacitance loads and each is composed of a series-feedback, low-noise amplifier, a unity-gain, shunt-feedback amplifier whose output is connected through a feedback capacitor to the series-feedback amplifier input. The stabilized capacitance loading of the anode allows distributed RC-line position encoding and subsequent time difference decoding by sensing the difference in rise times of pulses at the anode ends where the difference is primarily in response to the distributed capacitance along the anode. This allows the use of lower resistance wire anodes for spatial radiation detection which simplifies the counter construction and handling of the anodes, and stabilizes the anode resistivity at high count rates (>10.sup.6 counts/sec).

  10. Experience with position-sensitive neutron detectors at the Intense Pulsed Neutron Source

    NASA Astrophysics Data System (ADS)

    Crawford, R. K.; Haumann, J. R.; Epperson, J. E.; Thiyagarajan, P.; Schultz, A. J.; Felcher, G. P.; Montague, D. G.; Dejus, R. J.

    1990-12-01

    At the Intense Pulsed Neutron Source (IPNS) at Argonne National Laboratory, pulses of protons accelerated in a synchrotron produce pulses of fast neutrons via the spallation process in an enriched uranium target. After moderation, the resulting pulses of slow neutrons are directed into beams which serve a variety of neutron-scattering instruments. Currently there are thirteen neutron-scattering instruments in operation or under development at IPNS, and six of these use position-sensitive neutron detectors (PSDs). These PSDs are: a 30 cm × 30 cm, ˜3 mm resolution, neutron Anger camera area PSD with 6Li-glass scintillator; a 2.5 cm diameter, ˜0.7 mm resolution, microchannel-plate area PSD with 6Li-glass scintillator; a 20 cm × 20 cm, ˜5 mm resolution, 3He proportional-counter area PSD; a 40 cm × 40 cm, ˜4 mm resolution, 3He proportional-counter area PSD; a flat 20 cm long, ˜1.6 mm resolution, 3He proportional-counter linear PSD; and 160 cylindrical 3He proportional-counter linear PSDs, each of which is 1.27 cm in diameter and 60 cm long and has ˜14 mm resolution. These detectors, in addition to being position-sensitive, resolve the time of the neutron capture with ˜1 μs precision for neutron time-of-flight measurements. This paper will discuss these various PSDs with emphasis on the instrumental specifications and the reasons for the selection of the different types of PSDs, and will also discuss the observed performances of these PSDs.

  11. Experience with position sensitive neutron detectors at the Intense Pulsed Neutron Source

    SciTech Connect

    Crawford, R.K.; Haumann, J.R.; Schultz, A.J.; Felcher, G.P.; Epperson, J.E.; Thiyagarajan, P.; Montague, D.G.; Dejus, R.J.

    1990-05-07

    At the Intense Pulsed Neutron Source (IPNS) pulses of protons accelerated in a synchrotron produce pulses of fast neutrons via the spallation process in an enriched uranium target. After moderation, the resulting pulses of slow neutrons are directed into beams which serve a variety of neutron scattering instruments. Currently there are thirteen neutron scattering instruments in operation or under development at IPNS, and six of these use position-sensitive neutron detectors (PSDs). These PSDs are: a 30 cm {times} 30 cm, {approximately}3 mm resolution, neutron Anger camera area PSD with {sup 6}Li-glass scintillator; a 2.5 cm dia, {approximately}0.7 mm resolution, microchannel-plate area PSD with {sup 6}Li-glass scintillator; a 20 cm {times} 20 cm, {approximately}5 mm resolution, {sup 3}He proportional counter area PSD; a 40 cm {times} 40 cm, {approximately}4 mm resolution, {sup 3}He proportional counter area PSD; a flat 20 cm long, {approximately}1.6 mm resolution, {sup 3}He proportional counter linear PSD; and 160 cylindrical {sup 3}He proportional counter linear PSDs, each of which is 1.27 cm in dia 60 cm long and has {approximately}14 mm resolution. These detectors, in addition to being position-sensitive, resolve the time of the neutron capture with {approximately}1 {mu}s precision for neutron time-of-flight measurements. This paper will discuss these various PSDs with emphasis on the instrumental specifications and the reasons for the selection of the different types of PSDs, and will also discuss the observed performances of these PSDs. 14 refs., 6 figs., 1 tab.

  12. (Development of recommendations in the area of ionizing and nonionizing radiations)

    SciTech Connect

    Not Available

    1990-01-01

    This document discusses progress made from March 1, 1990 to October 30, 1990 in terms of publication of reports. This subjects discussed are related to the fields of radiation protection and ionizing and nonionizing radiations. Topics discussed published works, reports in press, printer's manuscript preparation, and scientific committee activities. (KJD)

  13. Improvement of the position linearity in a comb-type one-dimensional position sensitive detector

    NASA Astrophysics Data System (ADS)

    Tang, Jiuyao; Huang, Meizhen; Kim, Hoseob

    2002-09-01

    In a conventional, strip-type one-dimensional (1-D) position sensitive detector (PSD) the sensitive area and the position resistance area are combined together, the contact structure of the device is handicapped, so its accuracy and linearity is affected adversely. The sensitive area and the position resistance area in a new, comb-type 1-D PSD are separated to become the comb teeth and the comb ridge area respectively, moreover the position resistance area is made very narrow, thus the doping uniformity of that area is greatly improved. On the other hand, its position resistance can be largely increased owing to its narrower shape, if doping level is kept the same, so the restriction that is imposed on the contact structure previously can be lifted. Our measurements made on a strip-type 1-D PSD and a comb type 1-D PSD confirmed this difference, and showed that the accuracy and linearity of the comb type 1-D PSD has been increased markedly, especially the RMS nonlinearity of the comb type 1-D PSD is reduced to 0.090% from that of the strip-type 1-D PSD, 0.94%.

  14. Position-sensitive CdTe detector using improved crystal growth method

    NASA Technical Reports Server (NTRS)

    1988-01-01

    The feasibility of developing a position-sensitive CdTe detector array for astronomical observations in the hard X-ray, soft gamma ray region is demonstrated. In principle, it was possible to improve the resolution capability for imaging measurements in this region by orders of magnitude over what is now possible through the use of CdTe detector arrays. The objective was to show that CdTe crystals of the quality, size and uniformity required for this application can be obtained with a new high pressure growth technique. The approach was to fabricate, characterize and analyze a 100 element square array and several single-element detectors using crystals from the new growth process. Results show that detectors fabricated from transversely sliced, 7 cm diameter wafers of CdTe exhibit efficient counting capability and a high degree of uniformity over their entire areas. A 100 element square array of 1 sq mm detectors was fabricated and operated.

  15. Continuous lateral gradients in film morphology for position sensitive detection and organic solar cell optimization

    NASA Astrophysics Data System (ADS)

    Campoy-Quiles, M.; Randon, V.; Mróz, M. M.; Jarzaguet, M.; Garriga, M.; Cabanillas-González, J.

    2013-07-01

    We present a method to fabricate binary organic donor and acceptor blends exhibiting a controlled lateral gradient in morphology. Upon combining photometry, ellipsometry and Xray maps together with photoinduced absorption measurements, we show how the gradual exposure to solvent vapor results in a varying degree of polymer crystallinity for the polythiophene/soluble fullerene system along one direction. These morphologically graded samples are characterized by a spectral photoresponse that depends on the specific location in the area of the device where the light beam impinges, a property that stands as proof-of-concept for position sensitive detection. Moreover, we demonstrate that the development of graded morphologies is an effective one-step method which allows for fast performance optimization of organic solar cells. Finally, the appropriateness of eight different solvents for morphology control via vapor annealing is evaluated in a time-effective way using the advanced method, which helps to identify boiling point and solubility as the key processing parameters.

  16. A zero dead-time multi-particle time and position sensitive detector based on correlation between brightness and amplitude

    NASA Astrophysics Data System (ADS)

    Urbain, X.; Bech, D.; Van Roy, J.-P.; Géléoc, M.; Weber, S. J.; Huetz, A.; Picard, Y. J.

    2015-02-01

    A new multi-particle time and position sensitive detector using only a set of microchannel plates, a waveform digitizer, a phosphor screen, and a CMOS camera is described. The assignment of the timing information, as taken from the microchannel plates by fast digitizing, to the positions, as recorded by the camera, is based on the COrrelation between the BRightness of the phosphor screen spots, defined as their integrated intensity and the Amplitude of the electrical signals (COBRA). Tests performed by observing the dissociation of HeH, the fragmentation of H3 into two or three fragments, and the photo-double-ionization of Xenon atoms are presented, which illustrate the performances of the COBRA detection scheme.

  17. A zero dead-time multi-particle time and position sensitive detector based on correlation between brightness and amplitude.

    PubMed

    Urbain, X; Bech, D; Van Roy, J-P; Géléoc, M; Weber, S J; Huetz, A; Picard, Y J

    2015-02-01

    A new multi-particle time and position sensitive detector using only a set of microchannel plates, a waveform digitizer, a phosphor screen, and a CMOS camera is described. The assignment of the timing information, as taken from the microchannel plates by fast digitizing, to the positions, as recorded by the camera, is based on the COrrelation between the BRightness of the phosphor screen spots, defined as their integrated intensity and the Amplitude of the electrical signals (COBRA). Tests performed by observing the dissociation of HeH, the fragmentation of H3 into two or three fragments, and the photo-double-ionization of Xenon atoms are presented, which illustrate the performances of the COBRA detection scheme.

  18. A zero dead-time multi-particle time and position sensitive detector based on correlation between brightness and amplitude

    SciTech Connect

    Urbain, X. Bech, D.; Van Roy, J.-P.; Géléoc, M.; Weber, S. J.

    2015-02-15

    A new multi-particle time and position sensitive detector using only a set of microchannel plates, a waveform digitizer, a phosphor screen, and a CMOS camera is described. The assignment of the timing information, as taken from the microchannel plates by fast digitizing, to the positions, as recorded by the camera, is based on the COrrelation between the BRightness of the phosphor screen spots, defined as their integrated intensity and the Amplitude of the electrical signals (COBRA). Tests performed by observing the dissociation of HeH, the fragmentation of H{sub 3} into two or three fragments, and the photo-double-ionization of Xenon atoms are presented, which illustrate the performances of the COBRA detection scheme.

  19. The variation of ionospheric slab thickness over equatorial ionization area crest region

    NASA Astrophysics Data System (ADS)

    Chuo, Y. J.

    2007-06-01

    The GPS-derived total electron content (TEC) and NmF2 are measured at the Chung-Li ionosonde station (24.9°N, 121°E) in order to study the variations in slab thickness (τ) of the ionosphere at low-latitudes ionosphere during 1996 1999, corresponding to half of the 23rd solar cycle. This study presents the diurnal, seasonal, and solar flux variations in τ for different solar phases. The seasonal variations show that the average daily value is greater during summer and the reverse is true during equinox in the equatorial ionization anomaly (EIA) region. Moreover, the τ values are greater during the daytime (0800 1600 LT) and nighttime (2000 0400 LT) for summer and winter, respectively. The diurnal variation shows two abnormal peaks that appear during the pre-sunrise and post-sunset hours. The peak values decrease as the sunspot number increases particularly for the pre-sunrise peak. Furthermore, the variation in the F-peak height (hpF2) indicates that a thermospheric wind toward the equator leads to an increase in hpF2 and an enhancement in τ during the pre-sunrise period. Furthermore, the study shows the variations of τ values for different geophysical conditions such as the geomagnetic storm and earthquake. A comprehensive discussion about the relation between τ and the geophysical events is provided in the paper.

  20. Precision X-ray Measurement of the Position Sensitivity of Graphene Field Effect Transistors

    SciTech Connect

    Cazalas, Edward; Sarker, Biddut K.; Moore, Michael; Childres, Isaac; Chen, Yong P.; Jovanovic, Igor

    2015-07-01

    We have been exploring the graphene field-effect transistor (GFET) as a platform for detection of ionizing radiation, whereby the detection is achieved indirectly by use of the field effect in graphene, which is induced by the generation and transport of ionized charge carriers in the underlying undoped semiconductor substrate. An important characteristic of such a detector is scalability to large areas. Previous experimental studies suggest that the effective area significantly exceeds the size of graphene for field effect-based architectures, and this is also predicted from the operational principle of these devices. We describe the results of the experimental studies of GFETs on silicon carbide (SiC) substrates by use a microbeam Xray facility, provided by the Advanced Photon Source at Argonne National Laboratory. The results confirm that the effective area of the GFET is significantly larger than that of graphene with response measured at distances as large as 1000 μm from 10-μm size graphene. A simple transport model has been developed and is used to explain the spatial dependence of the GFET response. (authors)

  1. Evaluation of Nanoporous Gold with Controlled Surface Structures for Laser Desorption Ionization (LDI) Analysis: Surface Area Versus LDI Signal Intensity

    NASA Astrophysics Data System (ADS)

    Jin, Jang Mi; Choi, Suhee; Kim, Young Hwan; Choi, Man Ho; Kim, Jongwon; Kim, Sunghwan

    2012-09-01

    The structural effect of a nanoporous gold (NPG) surface on the signal intensities of laser desorption ionization-mass spectrometry (LDI-MS) were investigated using NPG surfaces with controlled structures. The relationship between surface area and LDI efficiency was compared and evaluated. Comparisons between bare flat gold and NPG surfaces show that nanostructures increased LDI efficiency. We also found that the LDI signal decreased with increasing depth of nanoporous layers, thus increasing the surface area. This result agrees with a previous report (Shin J. A. et al., J. Am. Soc. Mass Spectrom. 2010, 21, 989) in which the LDI efficiency of small molecules decreased for ZnO wires with longer lengths. This observation was explained by the penetration and deposition of samples into locations inaccessible to photons because of structural screening. The LDI-MS analysis of oils with NPG surfaces (but without matrix) showed the same trend whereby the NPG with about a 200 nm depth of porous area showed the highest sensitivity. This study clearly shows that the active surface area for solution chemistry can differ from LDI-MS and that NPGs can function as a substrate for LDI oil analysis.

  2. Position-sensitive radiation monitoring (surface contamination monitor). Innovative technology summary report

    SciTech Connect

    Not Available

    1999-06-01

    The Shonka Research Associates, Inc. Position-Sensitive Radiation Monitor both detects surface radiation and prepares electronic survey map/survey report of surveyed area automatically. The electronically recorded map can be downloaded to a personal computer for review and a map/report can be generated for inclusion in work packages. Switching from beta-gamma detection to alpha detection is relatively simple and entails moving a switch position to alpha and adjusting the voltage level to an alpha detection level. No field calibration is required when switching from beta-gamma to alpha detection. The system can be used for free-release surveys because it meets the federal detection level sensitivity limits requires for surface survey instrumentation. This technology is superior to traditionally-used floor contamination monitor (FCM) and hand-held survey instrumentation because it can precisely register locations of radioactivity and accurately correlate contamination levels to specific locations. Additionally, it can collect and store continuous radiological data in database format, which can be used to produce real-time imagery as well as automated graphics of survey data. Its flexible design can accommodate a variety of detectors. The cost of the innovative technology is 13% to 57% lower than traditional methods. This technology is suited for radiological surveys of flat surfaces at US Department of Energy (DOE) nuclear facility decontamination and decommissioning (D and D) sites or similar public or commercial sites.

  3. IONIZATION CHAMBER

    DOEpatents

    Redman, W.C.; Shonka, F.R.

    1958-02-18

    This patent describes a novel ionization chamber which is well suited to measuring the radioactivity of the various portions of a wire as the wire is moved at a uniform speed, in order to produce the neutron flux traverse pattern of a reactor in which the wire was previously exposed to neutron radiation. The ionization chamber of the present invention is characterized by the construction wherein the wire is passed through a tubular, straight electrode and radiation shielding material is disposed along the wire except at an intermediate, narrow area where the second electrode of the chamber is located.

  4. Imaging and Timing Performance of 1cm × 1cm Position-sensitive Solid-state Photomultiplier

    PubMed Central

    Schmall, J.; Stapels, C.; Christian, J.; Cherry, S.; Squillante, M. R.; Shah, K.

    2014-01-01

    We have designed and built a large-area 1cm × 1cm position-sensitive solid-state photomultiplier (PS-SSPM) for use in detector design for medical imaging applications. Our new large-area PS-SSPM concept implements resistive network between the micro-pixels, which are photodiodes operated in Geiger mode, called Geiger Photodiodes (GPDs), to provide continuous position sensitivity. Here we present imaging and timing performance of the large-area PS-SSPM for different temperatures and operating biases to find the optimum operating parameters for the device in imaging applications. A detector module was built by coupling a polished 8×8 LYSO array, with 1×1×20 mm3 elements, to a 1×1 cm2 PS-SSPM. Flood images recorded at room temperature show good crystal separation as all 64 elements were separated from each other. Cooling the device at 10 °C showed significant improvement. The device optimum bias voltage was ~4.5V over breakdown voltage. The coincidence timing resolution was improved significantly by increasing the operating bias, as well as by lowering the temperature to 0 °C. Results show excellent imaging performance and good timing response with a large-area PS-SSPM device. PMID:25540669

  5. CdZnTe position-sensitive drift detectors with thicknesses up to 5 cm

    SciTech Connect

    Bolotnikov, A. E. Camarda, G. S.; Cui, Y.; Gul, R.; De Geronimo, G.; Fried, J.; Hossain, A.; Vernon, E.; Yang, G.; James, R. B.; Chen, E.; MacKenzie, J. M.; Taherion, S.; El-hanany, U.; Cheng, S.; Gallagher, R.; Dedic, V.; Ocampo Giraldo, L.; Sellin, P.

    2016-02-29

    We investigated the feasibility of long-drift-time CdZnTe (CZT) gamma-ray detectors, fabricated from CZT material produced by Redlen Technologies. CZT crystals with cross-section areas of 5 × 5 mm{sup 2} and 6 × 6 mm{sup 2} and thicknesses of 20-, 30-, 40-, and 50-mm were configured as 3D position-sensitive drift detectors and were read out using a front-end ASIC. By correcting the electron charge losses caused by defects in the crystals, we demonstrated high performance for relatively thick detectors fabricated from unselected CZT material.

  6. Development of Position-Sensitive Magnetic Calorimeters for X-Ray Astronomy

    NASA Technical Reports Server (NTRS)

    Bandler, SImon; Stevenson, Thomas; Hsieh, Wen-Ting

    2011-01-01

    Metallic magnetic calorimeters (MMC) are one of the most promising devices to provide very high energy resolution needed for future astronomical x-ray spectroscopy. MMC detectors can be built to large detector arrays having thousands of pixels. Position-sensitive magnetic (PoSM) microcalorimeters consist of multiple absorbers thermally coupled to one magnetic micro calorimeter. Each absorber element has a different thermal coupling to the MMC, resulting in a distribution of different pulse shapes and enabling position discrimination between the absorber elements. PoSMs therefore achieve the large focal plane area with fewer number of readout channels without compromising spatial sampling. Excellent performance of PoSMs was achieved by optimizing the designs of key parameters such as the thermal conductance among the absorbers, magnetic sensor, and heat sink, as well as the absorber heat capacities. Micro fab ri - cation techniques were developed to construct four-absorber PoSMs, in which each absorber consists of a two-layer composite of bismuth and gold. The energy resolution (FWHM full width at half maximum) was measured to be better than 5 eV at 6 keV x-rays for all four absorbers. Position determination was demonstrated with pulse-shape discrimination, as well as with pulse rise time. X-ray microcalorimeters are usually designed to thermalize as quickly as possible to avoid degradation in energy resolution from position dependence to the pulse shapes. Each pixel consists of an absorber and a temperature sensor, both decoupled from the cold bath through a weak thermal link. Each pixel requires a separate readout channel; for instance, with a SQUID (superconducting quantum interference device). For future astronomy missions where thousands to millions of resolution elements are required, having an individual SQUID readout channel for each pixel becomes difficult. One route to attaining these goals is a position-sensitive detector in which a large continuous or

  7. Theoretical Noise Analysis on a Position-sensitive Metallic Magnetic Calorimeter

    NASA Technical Reports Server (NTRS)

    Smith, Stephen J.

    2007-01-01

    We report on the theoretical noise analysis for a position-sensitive Metallic Magnetic Calorimeter (MMC), consisting of MMC read-out at both ends of a large X-ray absorber. Such devices are under consideration as alternatives to other cryogenic technologies for future X-ray astronomy missions. We use a finite-element model (FEM) to numerically calculate the signal and noise response at the detector outputs and investigate the correlations between the noise measured at each MMC coupled by the absorber. We then calculate, using the optimal filter concept, the theoretical energy and position resolution across the detector and discuss the trade-offs involved in optimizing the detector design for energy resolution, position resolution and count rate. The results show, theoretically, the position-sensitive MMC concept offers impressive spectral and spatial resolving capabilities compared to pixel arrays and similar position-sensitive cryogenic technologies using Transition Edge Sensor (TES) read-out.

  8. A study of the timing properties of position-sensitive avalanche photodiodes

    PubMed Central

    Wu, Yibao; Ng, Thomas SC; Yang, Yongfeng; Shah, Kanai; Farrell, Richard; Cherry, Simon R

    2009-01-01

    In this paper we study position-dependent timing shifts and timing resolution in position sensitive avalanche photodiodes (PSAPDs) and their effect on the coincidence window used in positron emission tomography (PET) systems using these devices. There is a delay in PSAPD signals that increases as the excitation position moves from the corner to the center of the device and the timing resolution concurrently worsens. The difference in timing between the center and corner can be up to 30.7 ns for a 14×14 mm2 area PSAPD. This means that a PSAPD-based PET system could require a very wide coincidence timing window (>60 ns) if this effect is not corrected, although the individual crystal pairs still have full-width half-maximum (FWHM) timing resolutions better than 7.4 ns. In addition to characterizing the timing properties of PSAPDs, two correction methods were developed and applied to data from a pair of PSAPD detectors. These two timing offset corrections reduced the timing shift of a crystal pair from 52.4 ns to 9.7 ns or 1.3 ns, improved FWHM timing resolution of the detector pair from 24.6 ns to 9.5 ns or 6.0 ns and reduced the timing window (sufficient to cover at least twice the FWHM for all crystal pairs) from 65.1 ns to 22.0 ns or 15.2 ns respectively. A two-step timing alignment method is proposed for a PET system consisting of multiple PSAPDs. Lastly, the effect of PSAPD size on the timing performance was also evaluated. PMID:19671971

  9. A study of the timing properties of position-sensitive avalanche photodiodes.

    PubMed

    Wu, Yibao; Ng, Thomas S C; Yang, Yongfeng; Shah, Kanai; Farrell, Richard; Cherry, Simon R

    2009-09-07

    In this paper, we study position-dependent timing shifts and timing resolution in position sensitive avalanche photodiodes (PSAPDs) and their effects on the coincidence window used in positron emission tomography (PET) systems using these devices. There is a delay in PSAPD signals that increases as the excitation position moves from the corner to the center of the device and the timing resolution concurrently worsens. The difference in timing between the center and the corner can be up to 30.7 ns for a 14 x 14 mm(2) area PSAPD. This means that a PSAPD-based PET system could require a very wide coincidence timing window (>60 ns) if this effect is not corrected, although the individual crystal pairs still have full-width half-maximum (FWHM) timing resolutions better than 7.4 ns. In addition to characterizing the timing properties of PSAPDs, two correction methods were developed and applied to data from a pair of PSAPD detectors. These two timing offset corrections reduced the timing shift of a crystal pair from 52.4 ns to 9.7 ns or 1.3 ns, improved the FWHM timing resolution of the detector pair from 24.6 ns to 9.5 ns or 6.0 ns and reduced the timing window (sufficient to cover at least twice the FWHM for all crystal pairs) from 65.1 ns to 22.0 ns or 15.2 ns, respectively. A two-step timing alignment method is proposed for a PET system consisting of multiple PSAPDs. Lastly, the effect of PSAPD size on the timing performance was also evaluated.

  10. Theory and Development of Position-Sensitive Quantum Calorimeters. Degree awarded by Stanford Univ.

    NASA Technical Reports Server (NTRS)

    Figueroa-Feliciano, Enectali; White, Nicholas E. (Technical Monitor)

    2001-01-01

    Quantum calorimeters are being developed as imaging spectrometers for future X-ray astrophysics observatories. Much of the science to be done by these instruments could benefit greatly from larger focal-plane coverage of the detector (without increasing pixel size). An order of magnitude more area will greatly increase the science throughput of these future instruments. One of the main deterrents to achieving this goal is the complexity of the readout schemes involved. We have devised a way to increase the number of pixels from the current baseline designs by an order of magnitude without increasing the number of channels required for readout. The instrument is a high energy resolution, distributed-readout imaging spectrometer called a Position-Sensitive Transition-Edge Sensor (POST). A POST is a quantum calorimeter consisting of two Transition-Edge Sensors (TESS) on the ends of a long absorber capable of one-dimensional imaging spectroscopy. Comparing rise time and energy information from the two TESS, the position of the event in the POST is determined. The energy of the event is inferred from the sum of the two pulses. We have developed a generalized theoretical formalism for distributed-readout calorimeters and apply it to our devices. We derive the noise theory and calculate the theoretical energy resolution of a POST. Our calculations show that a 7-pixel POST with 6 keV saturation energy can achieve 2.3 eV resolution, making this a competitive design for future quantum calorimeter instruments. For this thesis we fabricated 7- and 15-pixel POSTS using Mo/Au TESs and gold absorbers, and moved from concept drawings on scraps of napkins to a 32 eV energy resolution at 1.5 keV, 7-pixel POST calorimeter.

  11. A novel position-sensitive mega-size dosimeter for photoneutrons in high-energy X-ray medical accelerators.

    PubMed

    Sohrabi, Mehdi; Hakimi, Amir; Mahdavi, Seyed Rabi

    2016-06-01

    A novel position-sensitive mega-size polycarbonate (MSPC) dosimeter is introduced. It provides photoneutron (PN) dose equivalent matrix of positions in and out of a beam of a high energy X-ray medical accelerator under a single exposure. A novel position-sensitive MSPC dosimeter was developed and applied. It has an effective etched area of 50×50cm(2), as used in this study, processed in a mega-size electrochemical etching chamber to amplify PN-induced-recoil tracks to a point viewed by the unaided eyes. Using such dosimeters, PN dose equivalents, dose equivalent profiles and isodose equivalent distribution of positions in and out of beams for different X-ray doses and field sizes were determined in a Siemens ONCOR Linac. The PN dose equivalent at each position versus X-ray dose was linear up to 20Gy studied. As the field size increased, the PN dose equivalent in the beam was also increased but it remained constant at positions out of the beam up to 20cm away from the beam edge. The jaws and MLCs due to material differences and locations relative to the target produce different PN contributions. The MSPC dosimeter introduced in this study is a perfect candidate for PN dosimetry with unique characteristics such as simplicity, efficiency, dose equivalent response, large size, flexibility to be bent, resembling the patient's skin, highly position-sensitive with high spatial resolution, highly insensitive to X-rays, continuity in measurements and need to a single dosimeter to obtain PN dose equivalent matrix data under a single X-ray exposure. Copyright © 2016 Associazione Italiana di Fisica Medica. Published by Elsevier Ltd. All rights reserved.

  12. Properties of large area ErBa2Cu3O(7-x) thin films deposited by ionized cluster beams

    NASA Technical Reports Server (NTRS)

    Levenson, L. L.; Stan, Mark A.; Bhasin, Kul B.

    1991-01-01

    ErBa2Cu3O(7-x) films have been produced by simultaneous deposition of Er, Ba, and Cu from three ionized cluster beam (ICB) sources at acceleration voltages of 0.3 to 0.5 kV. Combining ozone oxidation with ICB deposition at 650 C eliminated any need of post annealing processing. The substrates were rotated at 10 rotations per minute during the deposition which took place at a rate of about 3 to 4 nm. Films with areas up to 70 mm in diameter have been made by ICB deposition. These films, 100 nm thick, were deposited on SrTiO3 (100) substrates at 650 C in a mixture of six percent O3 in O2 at a total pressure of 4 x 10(exp -4) Torr. They had T(sub c) ranging from 84.3 K to 86.8 K over a 70 mm diameter and J(sub c) above 10(exp 6) A/sq cm at 77 K. X ray diffraction measurements of the three samples showed preferential c-axis orientation normal to the substrate surface. Scanning electron micrographs (SEM) of the three samples also show some texture dependence on sample position. For the three samples, there is a correlation between SEM texture, full width at half-maximum of rocking curves and J(sub c) versus temperature curves.

  13. GREATS: GOODS Re-ionization Era wide-Area Treasury: emission lines, SFRs, and stellar masses at z > 7

    NASA Astrophysics Data System (ADS)

    Labbe, Ivo

    2015-08-01

    Joint HST/WFC3 and Spitzer/IRAC observations are a powerful probe of the build up of galaxies in the early universe z > 4. A particularly surprising result in recent years has been the discovery of ubiquitous strong nebular emission lines in bright 4 < z < 8 galaxies. It is well understood that these strongly affect fundamental estimates, such as stellar mass. But apart from being a nuisance they also carry valuable information and allow us to study the SFR distribution and dust attenuation, while improving photometric redshifts and constraining ionisation properties. With IRAC programs over the Hubble Frontier Fields beginning to explore the ultra faint end L << L*, I will introduce GREATS: GOODS Re-ionization Era wide-Area Treasury from Spitzer, the 730 hour cycle-11 exploration ultradeep Spitzer/IRAC program over GOODS-North and GOODS-South to characterise the properties of normal L* galaxies at z > 7. Combined with techniques to select ultra bright high-z galaxies using IRAC over the widest fields, we are now for the first time in a position to constrain both the bright, medium, and faint end of the mass function at z > 7.

  14. Complex microcalorimeter models and their application to position-sensitive detectors

    SciTech Connect

    Figueroa-Feliciano, Enectali

    2006-06-01

    We present a general formalism for calculating the linear response, noise spectrum, and energy resolution of complex calorimeters. Using this formalism calorimeters with arbitrary numbers of distinct linked heat capacity systems and/or coupled thermometers can be analyzed. We use this formalism to derive the theoretical resolution of an imaging microcalorimeter called a position- sensitive transition-edge sensor.

  15. A Study of Position-Sensitive Solid-State Photomultiplier Signal Properties.

    PubMed

    Schmall, Jeffrey P; Du, Junwei; Judenhofer, Martin S; Dokhale, Purushottam; Christian, James; McClish, Mickel; Shah, Kanai S; Cherry, Simon R

    2014-06-12

    We present an analysis of the signal properties of a position-sensitive solid-state photomultiplier (PS-SSPM) that has an integrated resistive network for position sensing. Attractive features of PS-SSPMs are their large area and ability to resolve small scintillator crystals. However, the large area leads to a high detector capacitance, and in order to achieve high spatial resolution a large network resistor value is required. These inevitably create a low-pass filter that drastically slows what would be a fast micro-cell discharge pulse. Significant changes in the signal shape of the PS-SSPM cathode output as a function of position are observed, which result in a position-dependent time delay when using traditional time pick-off methods such as leading edge discrimination and constant fraction discrimination. The timing resolution and time delay, as a function of position, were characterized for two different PS-SSPM designs, a continuous 10 mm × 10 mm PS-SSPM and a tiled 2 × 2 array of 5 mm × 5 mm PS-SSPMs. After time delay correction, the block timing resolution, measured with a 6 × 6 array of 1.3 × 1.3 × 20 mm(3) LSO crystals, was 8.6 ns and 8.5 ns, with the 10 mm PS-SSPM and 5 mm PS-SSPM respectively. The effect of crystal size on timing resolution was also studied, and contrary to expectation, a small improvement was measured when reducing the crystal size from 1.3 mm to 0.5 mm. Digital timing methods were studied and showed great promise for allowing accurate timing by implementation of a leading edge time pick-off. Position-dependent changes in signal shape on the anode side also are present, which complicates peak height data acquisition methods used for positioning. We studied the effect of trigger position on signal amplitude, flood histogram quality, and depth-of-interaction resolution in a dual-ended readout detector configuration. We conclude that detector timing and positioning can be significantly improved by implementation of digital timing

  16. A Simple Capacitive Charge-Division Readout for Position-Sensitive Solid-State Photomultiplier Arrays

    PubMed Central

    Du, Junwei; Schmall, Jeffrey P.; Yang, Yongfeng; Di, Kun; Dokhale, Purushottam A.; Shah, Kanai S.; Cherry, Simon R.

    2014-01-01

    A capacitive charge-division readout method for reading out a 2 × 2 array of 5 mm × 5 mm position-sensitive solid-state photomultipliers (PS-SSPM) was designed and evaluated. Using this analog multiplexing method, the 20 signals (16 position, 4 timing) from the PS-SSPM array are reduced to 5 signals (4 position, 1 timing), allowing the PS-SSPM array to be treated as an individual large-area PS-SSPM module. A global positioning approach can now be used, instead of individual positioning for each PS-SSPM in the array, ensuring that the entire light signal is utilized. The signal-to-noise ratio (SNR) and flood histogram quality at different bias voltages (27.5 V to 32.0 V at 0.5 V intervals) and a fixed temperature of 0 °C were evaluated by coupling a 6 × 6 array of 1.3 mm × 1.3 mm × 20 mm polished LSO crystals to the center of the PS-SSPM array. The timing resolution was measured at a fixed bias voltage of 31.0 V and a fixed temperature of 0 °C. All the measurements were evaluated and compared using capacitors with different values and tolerances. Capacitor values ranged from 0.051 nf to 10 nf, and the capacitance tolerance ranged from 1% to 20%. The results show that better performance was achieved using capacitors with smaller values and better capacitance tolerance. Using 0.2 nf capacitors, the SNR, energy resolution and timing resolution were 24.3, 18.2% and 8.8 ns at a bias voltage 31.0 V, respectively. The flood histogram quality was also evaluated by using a 10 × 10 array of 1 mm × 1 mm × 10 mm polished LSO crystals and a 10 × 10 array of 0.7 mm × 0.7 mm × 20 mm unpolished LSO crystals to determine the smallest crystal size resolvable. These studies showed that the high spatial resolution of the PS-SSPM was preserved allowing for 0.7 mm crystals to be identified. These results show that the capacitive charge-division analog signal processing method can significantly reduce the number of electronic channels, from 20 to 5, while retaining the

  17. Position sensitivity in large spectroscopic LaBr3:Ce crystals for Doppler broadening correction

    NASA Astrophysics Data System (ADS)

    Blasi, N.; Giaz, A.; Boiano, C.; Brambilla, S.; Camera, F.; Million, B.; Riboldi, S.

    2016-12-01

    The position sensitivity of a large LaBr3:Ce crystal was investigated with the aim of correcting for the Doppler broadening in nuclear physics experiments. The crystal was cylindrical, 3 in×3 in (7.62 cm x 7.62 cm) and with diffusive surfaces as typically used in nuclear physics basic research to measure medium or high energy gamma rays (0.5 MeVPosition Sensitive Photomultipliers (PSPMT). The signals from the 256 segments of the four PSPMTs were acquired grouping them into 16 elements. An event by event analysis was performed and a positon resolution of the order of 2 cm was found. It was verified that this allows an important reduction of the Doppler broadening induced by relativistic beams in Nuclear Physics experiments.

  18. Time of flight elastic recoil detection analysis with a position sensitive detector

    SciTech Connect

    Siketic, Zdravko; Radovic, Iva Bogdanovic; Jaksic, Milko; Skukan, Natko

    2010-03-15

    A position sensitive detection system based on the microchannel plate detector has been constructed and installed at the existing time of flight (TOF) spectrometer in order to perform a kinematic correction and improve the surface time/depth resolution of elastic recoil detection analysis (ERDA) system. The position resolution of the detector has been tested for different types of ions and anode voltages. TOF spectra of recoiled O ions from SiO{sub 2} and F from CaF{sub 2} were collected in coincidence with position sensitive detector signal. Kinematic correction of TOF spectra improved surface time/depth resolution by {approx}20% for our system; however even higher improvements could be obtained in larger solid angle TOF-ERDA systems.

  19. Powder diffraction by fixed incident angle reflection using a curved position-sensitive detector

    SciTech Connect

    Haggerty, Ryan P.; Sarin, Pankaj; Bérar, Jean-Francois; Apostolov, Zlatomir D.; Kriven, Waltraud M.

    2010-05-25

    As curved position-sensitive detectors improve in angular resolution, the effects that fixed incident angle reflection have on X-ray diffraction peaks become more apparent. In this study the effects of sample transparency, incident beam height, detector resolution and sample displacement on the intensity, location, width and shape of powder diffraction peaks were examined. The functions describing each of these phenomena are presented and were successfully used to quantitatively model the diffraction peaks collected in this geometry. Three distinct regimes of diffraction peak resolution were identified from the phenomena that limit the peak variance. Pertinent criteria based on experimental parameters have been outlined to classify fixed incident angle reflection experiments into each regime. Guidelines for improvement of experimental resolution and for conducting analysis of data acquired using fixed incident angle reflection geometry and curved position-sensitive detectors are also provided.

  20. Position-sensitive detection of slow neutrons: Survey of fundamental principles

    SciTech Connect

    Crawford, R.K.

    1992-01-01

    This paper sets forth the fundamental principles governing the development of position-sensitive detection systems for slow neutrons. Since neutrons are only weakly interacting with most materials, it is not generally practical to detect slow neutrons directly. Therefore all practical slow neutron detection mechanisms depend on the use of nuclear reactions to convert'' the neutron to one or more charged particles, followed by the subsequent detection of the charged particles. The different conversion reactions which can be used are discussed, along with the relative merits of each. This is followed with a discussion of the various methods of charged particle detection, how these lend themselves to position-sensitive encoding, and the means of position encoding which can be applied to each case. Detector performance characteristics which may be of importance to the end user are discussed and related to these various detection and position-encoding mechanisms.

  1. Position-sensitive detection of slow neutrons: Survey of fundamental principles

    SciTech Connect

    Crawford, R.K.

    1992-07-01

    This paper sets forth the fundamental principles governing the development of position-sensitive detection systems for slow neutrons. Since neutrons are only weakly interacting with most materials, it is not generally practical to detect slow neutrons directly. Therefore all practical slow neutron detection mechanisms depend on the use of nuclear reactions to ``convert`` the neutron to one or more charged particles, followed by the subsequent detection of the charged particles. The different conversion reactions which can be used are discussed, along with the relative merits of each. This is followed with a discussion of the various methods of charged particle detection, how these lend themselves to position-sensitive encoding, and the means of position encoding which can be applied to each case. Detector performance characteristics which may be of importance to the end user are discussed and related to these various detection and position-encoding mechanisms.

  2. Fuel cell with ionization membrane

    NASA Technical Reports Server (NTRS)

    Hartley, Frank T. (Inventor)

    2007-01-01

    A fuel cell is disclosed comprising an ionization membrane having at least one area through which gas is passed, and which ionizes the gas passing therethrough, and a cathode for receiving the ions generated by the ionization membrane. The ionization membrane may include one or more openings in the membrane with electrodes that are located closer than a mean free path of molecules within the gas to be ionized. Methods of manufacture are also provided.

  3. DETECTORS AND EXPERIMENTAL METHODS: New test and analysis of position-sensitive-silicon-detector

    NASA Astrophysics Data System (ADS)

    Feng, Lang; Ge, Yu-Cheng; Wang, He; Fan, Feng-Ying; Qiao, Rui; Lu, Fei; Song, Yu-Shou; Zheng, Tao; Ye, Yan-Lin

    2009-01-01

    We have tested and analyzed the properties of two-dimensional Position-Sensitive-silicon-Detector (PSD) with new integrated preamplifiers. The test demonstrates that the best position resolution for 5.5 MeV α particles is 1.7 mm (FWHM), and the best energy resolution is 2.1%, which are notably better than the previously reported results. A scaling formula is introduced to make the absolute position calibration.

  4. A position-sensitive X-ray detector for the HEAO-A satellite.

    NASA Technical Reports Server (NTRS)

    Held, D.; Weisskopf, M. C.

    1973-01-01

    A position-sensitive, low-energy proportional counter system is described which will be used on the High-Energy Astronomical Observatory, Mission A, spacecraft. The associated system incorporates the capability to employ pulse-shape discrimination for background rejection and interpolation circuitry to locate the centroid of an X-ray event with an accuracy of approximately one eighth the cathode-wire spacing.

  5. Implementation of Complex Signal Processing Algorithms for Position-Sensitive Microcalorimeters

    NASA Technical Reports Server (NTRS)

    Smith, Stephen J.

    2008-01-01

    We have recently reported on a theoretical digital signal-processing algorithm for improved energy and position resolution in position-sensitive, transition-edge sensor (POST) X-ray detectors [Smith et al., Nucl, lnstr and Meth. A 556 (2006) 2371. PoST's consists of one or more transition-edge sensors (TES's) on a large continuous or pixellated X-ray absorber and are under development as an alternative to arrays of single pixel TES's. PoST's provide a means to increase the field-of-view for the fewest number of read-out channels. In this contribution we extend the theoretical correlated energy position optimal filter (CEPOF) algorithm (originally developed for 2-TES continuous absorber PoST's) to investigate the practical implementation on multi-pixel single TES PoST's or Hydras. We use numerically simulated data for a nine absorber device, which includes realistic detector noise, to demonstrate an iterative scheme that enables convergence on the correct photon absorption position and energy without any a priori assumptions. The position sensitivity of the CEPOF implemented on simulated data agrees very well with the theoretically predicted resolution. We discuss practical issues such as the impact of random arrival phase of the measured data on the performance of the CEPOF. The CEPOF algorithm demonstrates that full-width-at- half-maximum energy resolution of < 8 eV coupled with position-sensitivity down to a few 100 eV should be achievable for a fully optimized device.

  6. Commissioning of a PTW 34070 large-area plane-parallel ionization chamber for small field megavoltage photon dosimetry.

    PubMed

    Kupfer, Tom; Lehmann, Joerg; Butler, Duncan J; Ramanathan, Ganesan; Bailey, Tracy E; Franich, Rick D

    2017-10-04

    This study investigates a large-area plane-parallel ionization chamber (LAC) for measurements of dose-area product in water (DAPw ) in megavoltage (MV) photon fields. Uniformity of electrode separation of the LAC (PTW34070 Bragg Peak Chamber, sensitive volume diameter: 8.16 cm) was measured using high-resolution microCT. Signal dependence on angle α of beam incidence for square 6 MV fields of side length s = 20 cm and 1 cm was measured in air. Polarity and recombination effects were characterized in 6, 10, and 18 MV photons fields. To assess the lateral setup tolerance, scanned LAC profiles of a 1 × 1 cm(2) field were acquired. A 6 MV calibration coefficient, ND,w,LAC , was determined in a field collimated by a 5 cm diameter stereotactic cone with known DAPw . Additional calibrations in 10 × 10 cm(2) fields at 6, 10, and 18 MV were performed. Electrode separation is uniform and agrees with specifications. Volume-averaging leads to a signal increase proportional to ~1/cos(α) in small fields. Correction factors for polarity and recombination range between 0.9986 to 0.9996 and 1.0007 to 1.0024, respectively. Off-axis displacement by up to 0.5 cm did not change the measured signal in a 1 × 1 cm(2) field. ND,w,LAC was 163.7 mGy cm(-2) nC(-1) and differs by +3.0% from the coefficient derived in the 10 × 10 cm(2) 6 MV field. Response in 10 and 18 MV fields increased by 1.0% and 2.7% compared to 6 MV. The LAC requires only small correction factors for DAPw measurements and shows little energy dependence. Lateral setup errors of 0.5 cm are tolerated in 1 × 1 cm(2) fields, but beam incidence must be kept as close to normal as possible. Calibration in 10 × 10 fields is not recommended because of the LAC's over-response. The accuracy of relative point-dose measurements in the field's periphery is an important limiting factor for the accuracy of DAPw measurements. © 2017 The Authors. Journal of Applied Clinical Medical Physics published by Wiley Periodicals, Inc. on

  7. Effects of dose and of partial body ionizing radiation on taste aversion learning in rats with lesions of the area postrema

    SciTech Connect

    Rabin, B.M.; Hunt, W.A.; Lee, J. )

    1984-01-01

    The effect of area postrema lesions on the acquisition of a conditioned taste aversion following partial body exposure to ionizing radiation was investigated in rats exposed to head-only irradiation at 100, 200 and 300 rad or to body-only irradiation at 100 and 200 rad. Following head-only irradiation area postrema lesions produced a significant attenuation of the radiation-induced taste aversion at all dose levels, although the rats still showed a significant reduction in sucrose preference. Following body-only exposure, area postrema lesions completely disrupted the acquisition of the conditioned taste aversion. The results are interpreted as indicating that: (a) the acquisition of a conditioned taste aversion following body-only exposure is mediated by the area postrema; and (b) taste aversion learning following radiation exposure to the head-only is mediated by both the area postrema and a mechanism which is independent of the area postrema.

  8. Thermal Neutron Imaging Using A New Pad-Based Position Sensitive Neutron Detector

    SciTech Connect

    Dioszegi I.; Vanier P.E.; Salwen C.; Chichester D.L.; Watson S.M.

    2016-10-29

    Thermal neutrons (with mean energy of 25 meV) have a scattering mean free path of about 20 m in air. Therefore it is feasible to find localized thermal neutron sources up to ~30 m standoff distance using thermal neutron imaging. Coded aperture thermal neutron imaging was developed in our laboratory in the nineties, using He-3 filled wire chambers. Recently a new generation of coded-aperture neutron imagers has been developed. In the new design the ionization chamber has anode and cathode planes, where the anode is composed of an array of individual pads. The charge is collected on each of the individual 5x5 mm2 anode pads, (48x48 in total, corresponding to 24x24 cm2 sensitive area) and read out by application specific integrated circuits (ASICs). The high sensitivity of the ASICs allows unity gain operation mode. The new design has several advantages for field deployable imaging applications, compared to the previous generation of wire-grid based neutron detectors. Among these are the rugged design, lighter weight and use of non-flammable stopping gas. For standoff localization of thermalized neutron sources a low resolution (11x11 pixel) coded aperture mask has been fabricated. Using the new larger area detector and the coarse resolution mask we performed several standoff experiments using moderated californium and plutonium sources at Idaho National Laboratory. In this paper we will report on the development and performance of the new pad-based neutron camera, and present long range coded-aperture images of various thermalized neutron sources.

  9. Evaluation of a position sensitive neutron detector based on Li6Gd(BO3)3 scintillator

    NASA Astrophysics Data System (ADS)

    Schooneveld, Erik M.; Czirr, J. B.; McKnight, Thomas K.; Rhodes, Nigel J.; Ibberson, R. M.

    2002-11-01

    As a result of the ever increasing demand for higher neutron flux, future neutron scintillator detectors will require faster scintillators with a high light yield and low gamma sensitivity. Initial measurements with single element prototypes demonstrated that the new lithium gadolinium borate (LiGdBO) scintillator, using 6Li as the neutron absorber, was a promising candidate. As a result of this work, a full size position sensitive detector module has been made consisting of 120 LiGdBO elements. This module was installed on the High Resolution Powder Diffractometer (HRPD) beam line at ISIS for evaluation. The LiGdBO detector has been constructed with the same geometry and theoretically the same neutron absorption efficiency as the existing HRPD ZnS scintillator detector modules. In this way it was possible to make a more exact comparison of the relative detector performances. Measurements have shown that the neutron energy resolution and detection efficiency of both types of detector are identical. Gamma sensitivity and quiet count rate are somewhat higher for the LiGdBO than the ZnS scintillator detector, but still at an acceptable level for many applications. The short decay time of the LiGdBO scintillator has enhanced the count-rate capability of the detector by an order of magnitude. These measurements show that realistic large area position sensitive neutron detectors can be fabricated with LiGdBO scintillator using an optical fibre readout. LiGdBO is thus a promising scintillator for future detectors at the new high flux facilities currently under construction.

  10. Position sensitive x-ray spectrophotometer using microwave kinetic inductance detectors

    SciTech Connect

    Mazin, Benjamin A.; Bumble, Bruce; Day, Peter K.; Eckart, Megan E.; Golwala, Sunil; Zmuidzinas, Jonas; Harrison, Fiona A.

    2006-11-27

    The surface impedance of a superconductor changes when energy is absorbed and Cooper pairs are broken to produce single electron (quasiparticle) excitations. This change may be sensitively measured using a thin-film resonant circuit called a microwave kinetic inductance detector (MKID). The practical application of MKIDs for photon detection requires a method of efficiently coupling the photon energy to the MKID. The authors present results on position sensitive x-ray detectors made by using two aluminum MKIDs on either side of a tantalum photon absorber strip. Diffusion constants, recombination times, and energy resolution are reported. MKIDs can easily be scaled into large arrays.

  11. Fast neutron spectrometry and dosimetry using a spherical moderator with position-sensitive detectors.

    PubMed

    Li, Taosheng; Yang, Lianzhen; Ma, Jizeng; Fang, Dong

    2007-01-01

    A neutron spectrometry and dosimetry measurement system has been developed based on a different design of the divided regions for a sphere, with three position-sensitive counters. The characteristics of the measurement system have been investigated in the reference radiation fields of Am-Be and (252)Cf sources. When realistic input spectra are used for the unfolding, the overall deviations of the calculated results for four dosimetric quantities are less than +/-10%. The results of other input spectra are also discussed in this report.

  12. Two-dimensional spectrally resolved position-sensitive proportional counter for plasma imaging

    SciTech Connect

    Thorn, D.; Beiersdorfer, P.

    2004-10-01

    We describe a 160x100 mm two-dimensional position-sensitive proportional counter for use in high-temperature plasma spectroscopy. The detector employs a novel design based on a printed circuit board for the cathode plane and a single-wire switchback design for the anode plane. The spacial resolution for one dimension is 200 {mu}m and for the other dimension is 2-5 mm. The integral nonlinearity is 0.08% for the first and 1% for the second dimension. We demonstrate the utility of the new detector with a spacially resolved measurement of the Lyman-{alpha} transitions in hydrogenic Ar{sup 17+}.

  13. Use of a pulsed magnetic field to increase the position sensitivity of a photomultiplier

    NASA Astrophysics Data System (ADS)

    Yong-Geng, Qian; Thompson, C. J.

    1987-05-01

    It is well known that photomultipliers (PMTs) are sensitive to external magnetic fields. We have used this property to vary the gain of the PMT depending on the position of the light source. Various coil configurations have been evaluated to produce local magnetic fields in the region between the photocathode and first dynode to maximize the amplitude variation in the anode signal with respect to change in the coil current. The aim was to improve the position sensitivity of a PMT used in positron emission tomography (PET). The position sensitivity was tested with an array of collimated light emitting diodes directed towards the photocathodes of a Hamamatsu R1548 PMT. The best coil position was above the photocathodes. A 60% reduction in output for light pulses from two LEDs near the coil was obtained with a current of 43 Ampere-turns while signals from two LEDs far from the coil remained the same. The rise time of the magnetic field was 2 μs.

  14. Position sensitivity in 3"×3" Spectroscopic LaBr3:Ce Crystals

    NASA Astrophysics Data System (ADS)

    Blasi, N.; Giaz, A.; Boiano, C.; Brambilla, S.; Camera, F.; Million, B.; Riboldi, S.

    2015-06-01

    The position sensitivity of a thick, cylindrical and continuous 3" × 3" (7.62 cm × 7.62 cm) LaBr3:Ce crystal with diffusive surfaces was investigated. Nuclear physics basic research uses thick LaBr3:Ce crystals (> 3cm) to measure medium or high energy gamma rays (0.5 MeV < Eγ< 20 MeV). In the first measurement the PMT photocathode entrance window was covered by black absorber except for a small window 1 cm × 1cm wide. A complete scan of the detector over a 0.5 cm step grid was performed. The data show that even in a 3" thick LaBr3:Ce crystal with diffusive surfaces the position of the full energy peak centroid depends on the source position. The position of the full energy peak centroids are sufficient to identify the collimated gamma source position. The crystal was then coupled to four Position Sensitive Photomultipliers (PSPMT). We acquired the signals from the 256 segments of the four PSPMTs grouping them into 16 elements. An event by event analysis shows a positon resolution of the order of 2 cm.

  15. Exploring the spatial resolution of position-sensitive microchannel plate detectors

    NASA Astrophysics Data System (ADS)

    Wiggins, Blake; Siwal, Davinder; Desouza, Romualdo

    2016-03-01

    High amplification and excellent timing make microchannel plate (MCP) detectors excellent devices for detection of photons, electrons, and ions. In addition to providing sub-nanosecond time resolution MCP detectors can also provide spatial resolution, thus making them useful in imaging applications. Use of a resistive anode (RA) is a routinely used approach to make an MCP position-sensitive. The spatial resolution of the RA associated with detection of a single incident electron was determined. Factors impacting the spatial resolution obtained with the RA will be discussed and the achieved spatial resolution of 64 μm (FWHM) will be presented. Recently, a novel approach has been developed to provide position-sensitivity for an MCP detector. In this approach, namely the induced signal approach, the position of the incident particle is determined by sensing the electron cloud emanating from a MCP stack. By utilizing the zero-crossing point of the inherently bipolar signals, a spatial resolution of 466 μm (FWHM) has been achieved. Work to improve the spatial resolution of the induced signal approach further will be presented. Supported by the US DOE NNSA under Award No. DE-NA0002012.

  16. An improved method of energy calibration for position-sensitive silicon detectors

    NASA Astrophysics Data System (ADS)

    Sun, Ming-Dao; Huang, Tian-Heng; Liu, Zhong; Ding, Bing; Yang, Hua-Bin; Zhang, Zhi-Yuan; Wang, Jian-Guo; Ma, Long; Yu, Lin; Wang, Yong-Sheng; Gan, Zai-Guo; Xiao-Hong, Zhou

    2016-04-01

    Energy calibration of resistive charge division-based position-sensitive silicon detectors is achieved by parabolic fitting in the traditional method, where the systematic variations of vertex and curvature of the parabola with energy must be considered. In this paper we extend the traditional method in order to correct the fitting function, simplify the procedure of calibration and improve the experimental data quality. Instead of a parabolic function as used in the traditional method, a new function describing the relation of position and energy is introduced. The energy resolution of the 8.088 MeV α decay of 213Rn is determined to be about 87 keV (FWHM), which is better than the result of the traditional method, 104 keV (FWHM). The improved method can be applied to the energy calibration of resistive charge division-based position-sensitive silicon detectors with various performances. Supported by ‘100 Person Project’ of the Chinese Academy of Sciences and the National Natural Science Foundation of China (11405224 and 11435014)

  17. Properties of large area ErBa2Cu3O(7-x) thin films deposited by ionized cluster beams

    NASA Technical Reports Server (NTRS)

    Levenson, L. L.; Stan, M.; Bhasin, K. B.

    1991-01-01

    Ionized cluster beam (ICB) deposition is employed to produce ErBa2Cu3O(7-x) films on different substrates without post-annealing. Films with diameters of up to 70 mm are grown on SrTiO3 100 plane and exhibit Tc values of 84-87 K, Jc of about 10 exp 6 A/sq m at 77 K. These films are epitaxial with the c-axis perpendicular to the plane of the substrate surface, and they can be routinely produced by ICB with good Jc and Tc.

  18. Position-sensitive detection of ultracold neutrons with an imaging camera and its implications to spectroscopy

    NASA Astrophysics Data System (ADS)

    Wei, Wanchun; Broussard, L. J.; Hoffbauer, M. A.; Makela, M.; Morris, C. L.; Tang, Z.; Adamek, E. R.; Callahan, N. B.; Clayton, S. M.; Cude-Woods, C.; Currie, S.; Dees, E. B.; Ding, X.; Geltenbort, P.; Hickerson, K. P.; Holley, A. T.; Ito, T. M.; Leung, K. K.; Liu, C.-Y.; Morley, D. J.; Ortiz, Jose D.; Pattie, R. W.; Ramsey, J. C.; Saunders, A.; Seestrom, S. J.; Sharapov, E. I.; Sjue, S. K.; Wexler, J.; Womack, T. L.; Young, A. R.; Zeck, B. A.; Wang, Zhehui

    2016-09-01

    Position-sensitive detection of ultracold neutrons (UCNs) is demonstrated using an imaging charge-coupled device (CCD) camera. A spatial resolution less than 15 μm has been achieved, which is equivalent to a UCN energy resolution below 2 pico-electron-volts through the relation δE =m0 gδx. Here, the symbols δE, δx, m0 and g are the energy resolution, the spatial resolution, the neutron rest mass and the gravitational acceleration, respectively. A multilayer surface convertor described previously is used to capture UCNs and then emits visible light for CCD imaging. Particle identification and noise rejection are discussed through the use of light intensity profile analysis. This method allows different types of UCN spectroscopy and other applications.

  19. Position-sensitive detection of ultracold neutrons with an imaging camera and its implications to spectroscopy

    DOE PAGES

    Wei, Wanchun; Broussard, Leah J.; Hoffbauer, Mark Arles; ...

    2016-05-16

    Position-sensitive detection of ultracold neutrons (UCNs) is demonstrated using an imaging charge-coupled device (CCD) camera. A spatial resolution less than 15μm has been achieved, which is equivalent to a UCN energy resolution below 2 pico-electron-volts through the relation δE=m0gδx. Here, the symbols δE, δx, m0 and g are the energy resolution, the spatial resolution, the neutron rest mass and the gravitational acceleration, respectively. A multilayer surface convertor described previously is used to capture UCNs and then emits visible light for CCD imaging. Particle identification and noise rejection are discussed through the use of light intensity profile analysis. As a result,more » this method allows different types of UCN spectroscopy and other applications.« less

  20. 3D scanning characteristics of an amorphous silicon position sensitive detector array system.

    PubMed

    Contreras, Javier; Gomes, Luis; Filonovich, Sergej; Correia, Nuno; Fortunato, Elvira; Martins, Rodrigo; Ferreira, Isabel

    2012-02-13

    The 3D scanning electro-optical characteristics of a data acquisition prototype system integrating a 32 linear array of 1D amorphous silicon position sensitive detectors (PSD) were analyzed. The system was mounted on a platform for imaging 3D objects using the triangulation principle with a sheet-of-light laser. New obtained results reveal a minimum possible gap or simulated defect detection of approximately 350 μm. Furthermore, a first study of the angle for 3D scanning was also performed, allowing for a broad range of angles to be used in the process. The relationship between the scanning angle of the incident light onto the object and the image displacement distance on the sensor was determined for the first time in this system setup. Rendering of 3D object profiles was performed at a significantly higher number of frames than in the past and was possible for an incident light angle range of 15 ° to 85 °.

  1. Position-sensitive detection of ultracold neutrons with an imaging camera and its implications to spectroscopy

    SciTech Connect

    Wei, Wanchun; Broussard, Leah J.; Hoffbauer, Mark Arles; Makela, Mark F.; Morris, Christopher L.; Tang, Zhaowen; Adamek, Evan Robert; Callahan, Nathen Brannan; Clayton, Steven M.; Cude-Woods, Chris B.; Currie, Scott Allister; Dees, E. B.; Ding, Xinjian; Geltenbort, Peter W.; Hickerson, Kevin Peter; Holley, Adam Tarte; Ito, Takeyasu M.; Leung, Kent Kwan Ho; Liu, Chen -Yu; Morley, Deborah Jean; Ortiz, Jose D.; Pattie, Jr., Robert Wayne; Ramsey, John Clinton; Saunders, Alexander; Seestrom, Susan Joyce; Sharapov, E. I.; Sjue, Sky K.; Wexler, Jonathan William; Womack, Todd Lane; Young, Albert Raymond; Zeck, Bryan Alexander; Wang, Zhehui

    2016-05-16

    Position-sensitive detection of ultracold neutrons (UCNs) is demonstrated using an imaging charge-coupled device (CCD) camera. A spatial resolution less than 15μm has been achieved, which is equivalent to a UCN energy resolution below 2 pico-electron-volts through the relation δE=m0gδx. Here, the symbols δE, δx, m0 and g are the energy resolution, the spatial resolution, the neutron rest mass and the gravitational acceleration, respectively. A multilayer surface convertor described previously is used to capture UCNs and then emits visible light for CCD imaging. Particle identification and noise rejection are discussed through the use of light intensity profile analysis. As a result, this method allows different types of UCN spectroscopy and other applications.

  2. Adhesion Force Measurements Using an Atomic Force Microscope Upgraded with a Linear Position Sensitive Detector

    PubMed Central

    Pierce, M.; Stuart, J.; Pungor, A.; Dryden, P.

    2012-01-01

    The atomic force microscope (AFM), in addition to providing images on an atomic scale, can be used to measure the forces between surfaces and the AFM probe. The potential uses of mapping the adhesive forces on the surface include a spatial determination of surface energy and a direct identification of surface proteins through specific protein–ligand binding interactions. The capabilities of the AFM to measure adhesive forces can be extended by replacing the four-quadrant photodiode detection sensor with an external linear position sensitive detector and by utilizing a dedicated user-programmable signal generator and acquisiton system. Such an upgrade enables the microscope to measure in the larger dynamic range of adhesion forces, improves the sensitivity and linearity of the measurement, and eliminates the problems inherent to the multiple repetitious contacts between the AFM probe and the specimen surface. PMID:25125792

  3. Position-sensitive detection of ultracold neutrons with an imaging camera and its implications to spectroscopy

    SciTech Connect

    Wei, Wanchun; Broussard, Leah J.; Hoffbauer, Mark Arles; Makela, Mark F.; Morris, Christopher L.; Tang, Zhaowen; Adamek, Evan Robert; Callahan, Nathen Brannan; Clayton, Steven M.; Cude-Woods, Chris B.; Currie, Scott Allister; Dees, E. B.; Ding, Xinjian; Geltenbort, Peter W.; Hickerson, Kevin Peter; Holley, Adam Tarte; Ito, Takeyasu M.; Leung, Kent Kwan Ho; Liu, Chen -Yu; Morley, Deborah Jean; Ortiz, Jose D.; Pattie, Jr., Robert Wayne; Ramsey, John Clinton; Saunders, Alexander; Seestrom, Susan Joyce; Sharapov, E. I.; Sjue, Sky K.; Wexler, Jonathan William; Womack, Todd Lane; Young, Albert Raymond; Zeck, Bryan Alexander; Wang, Zhehui

    2016-05-16

    Position-sensitive detection of ultracold neutrons (UCNs) is demonstrated using an imaging charge-coupled device (CCD) camera. A spatial resolution less than 15μm has been achieved, which is equivalent to a UCN energy resolution below 2 pico-electron-volts through the relation δE=m0gδx. Here, the symbols δE, δx, m0 and g are the energy resolution, the spatial resolution, the neutron rest mass and the gravitational acceleration, respectively. A multilayer surface convertor described previously is used to capture UCNs and then emits visible light for CCD imaging. Particle identification and noise rejection are discussed through the use of light intensity profile analysis. As a result, this method allows different types of UCN spectroscopy and other applications.

  4. Development of an optical lens based alpha-particle imaging system using position sensitive photomultiplier tube

    NASA Astrophysics Data System (ADS)

    Ando, Koki; Oka, Miki; Yamamoto, Seiichi

    2017-02-01

    We developed an optical lens based alpha-particle imaging system using position sensitive photomultiplier tube (PSPMT). The alpha-particle imaging system consists of an optical lens, an extension tube and a 1 in. square high quantum efficiency (HQE) type PSPMT. After a ZnS(Ag) is attached to subject, the scintillation image of ZnS(Ag) is focused on the photocathode of the PSPMT by the use of the optical lens. With this configuration we could image the alpha particle distribution with energy information without contacting to the subject. The spatial resolution and energy resolution were 0.8 mm FWHM and 50% FWHM at 5 mm from the optical lens, respectively. We could successfully image the alpha particle distribution in uranium ore. The developed alpha-particle imaging system will be a new tool for imaging alpha emitters with energy information without contacting the subject.

  5. High-Efficiency CdZnTe Position-Sensitive VFG Gamma-Ray Detectors for Safeguards Applications

    SciTech Connect

    Bolotnikov, Aleksey E.; James, Ralph B.; Cui, Y.; De Geronimo, G.; Vernon, E.; Camarda, G. S.; Hossain, A.; Yang, G.; Indusi, J.; Boyer, Brian

    2015-09-30

    The goal of this project is to incorporate a Cadmium-Zinc-Telluride (CdZnTe or CZT) detector (with 1% or better resolution) into a bench-top prototype for isotope identification and related safeguards applications. The bench-top system is based on a 2x2 array of 6x6x20 mm3 position-sensitive virtual Frisch-grid (VFG) CZT detectors. The key features of the array are that it allows for the use of average-grade CZT material with a moderate content of defects, and yet it provides high energy resolution, 1% FWHM at 662 keV, large effective area, and low-power consumption. The development of this type of 3D detector and new instruments incorporating them is motivated by the high cost and low availability of large, > 1 cm3, CZT crystals suitable for making multi-pixel detectors with acceptable energy resolution and efficiency.

  6. Position-sensitive change in the transition metal L-edge fine structures

    SciTech Connect

    Gulec, Ahmet; Phillips, Patrick J.; Klie, Robert F.

    2015-10-05

    Studying the structure and composition of solid-state materials on the atomic scale has become nearly routine in transmission electron microscopy with the development of novel electron optics and electron sources. In particular, with spatial resolutions better than 0.1 nm and energy resolution smaller than 100 meV, the stoichiometry, bonding, and coordination can now be examined on similar scales. Aberration-corrected scanning transmission electron microscopy and electron energy-loss spectroscopy (EELS) have played a crucial role in identifying charge ordering, valence, and as spin state transitions in transition metal perovskite oxides. In this letter, we investigate the effects of ever-decreasing electron-probe sizes on the measured near-edge fine-structure of the transition metal core-loss edge using EELS. We find that for certain transition metal perovskites, the position of the electron probe with respect to the atomic column is crucial in determining the correct valence state. Several reasons for the observed position-sensitive EELS fine-structure are discussed.

  7. Compton imaging with a highly-segmented, position-sensitive HPGe detector

    NASA Astrophysics Data System (ADS)

    Steinbach, T.; Hirsch, R.; Reiter, P.; Birkenbach, B.; Bruyneel, B.; Eberth, J.; Gernhäuser, R.; Hess, H.; Lewandowski, L.; Maier, L.; Schlarb, M.; Weiler, B.; Winkel, M.

    2017-02-01

    A Compton camera based on a highly-segmented high-purity germanium (HPGe) detector and a double-sided silicon-strip detector (DSSD) was developed, tested, and put into operation; the origin of γ radiation was determined successfully. The Compton camera is operated in two different modes. Coincidences from Compton-scattered γ-ray events between DSSD and HPGe detector allow for best angular resolution; while the high-efficiency mode takes advantage of the position sensitivity of the highly-segmented HPGe detector. In this mode the setup is sensitive to the whole 4π solid angle. The interaction-point positions in the 36-fold segmented large-volume HPGe detector are determined by pulse-shape analysis (PSA) of all HPGe detector signals. Imaging algorithms were developed for each mode and successfully implemented. The angular resolution sensitively depends on parameters such as geometry, selected multiplicity and interaction-point distances. Best results were obtained taking into account the crosstalk properties, the time alignment of the signals and the distance metric for the PSA for both operation modes. An angular resolution between 13.8° and 19.1°, depending on the minimal interaction-point distance for the high-efficiency mode at an energy of 1275 keV, was achieved. In the coincidence mode, an increased angular resolution of 4.6° was determined for the same γ-ray energy.

  8. The particle background of the Rosat PSPC. [Position Sensitive Proportional Counter

    NASA Technical Reports Server (NTRS)

    Snowden, S. L.; Plucinsky, P. P.; Briel, U.; Hasinger, G.; Pfeffermann, E.

    1992-01-01

    In order to permit quantitative studies of the diffuse cosmic X-ray background and of extended X-ray sources, the particle induced background of the Roentgen Satellite, Rosat, Position Sensitive Proportional Counter (PSPC) is parameterized. Data collected during 210,000 s of PSPC operation have been analyzed and the temporal, spectral, and spatial distributions investigated. About 77 percent of the residual events originate within the detector while the remainder enter through the counter window. During typical conditions, the count rate of the residual events is well correlated with the Master Veto (MV) count rate. The spectrum of these events is well described by a flat component plus a soft power law and an Al K-alpha line at 1.5 keV. Also during typical conditions, the ratio between the power law and flat components remains constant to +/- 4 while the relative Al K-alpha contribution increases with increasing MV count rate. The distribution of the counts over the field of view is uniform except for a slight radial dependence and shadowing caused by blockage of the externally produced component by the window support structure.

  9. Position-sensitive ``movie'' in situ neutron detector for the UCN τ experiment

    NASA Astrophysics Data System (ADS)

    Weaver, Hannah; UCNTau Collaboration

    2016-09-01

    Precision measurements of neutron β-decay parameters provide tests of fundamental theories in elementary particle physics and cosmology such as the Standard Model and Big Bang nucleosynthesis. In particular, the UCN τ experiment aims to measure the mean lifetime of ultracold neutrons confined in an asymmetric magneto-gravitational trap using an in situ neutron detector. This detector consists of a 20 nm film of 10B on top of a ZnS:Ag scintillating screen. The screen is readout using two photomultipliers which view an array of wavelength shifting fibers optically coupled to the scintillator. When the detector is lowered into the loaded trap, light is emitted due to the charged particles recoiling into the ZnS:Ag when neutrons absorb on the 10B. Phase space evolution in the stored neutron population can lead to apparent shifts in the measured neutron lifetime with the detector height. In order to quantify this systematic uncertainty, we are implementing a supplemental 64-channel position-sensitive PMT module with high quantum efficiency and fast time response to image the entire detector in situ during measurements. We have characterized a prototype using a ZnS screen and an α-particle source along with a prototype lens system and will report the results and future plans.

  10. ROSAT Position Sensitive Proportional Counter spectra of six Seyfert 1 galaxies

    NASA Technical Reports Server (NTRS)

    Turner, T. J.; George, I. M.; Mushotzky, R. F.

    1993-01-01

    We present the results from ROSAT Position Sensitive Proportional Counter observations of six Seyfert 1 galaxies in the soft (0.1-2.0 keV) X-ray band. The sources (Mrk 335, ESO 198-G24, ESO 141-G55, Mrk 509, NGC 7469, and MCG-2-58-22) were chosen to have low absorbing column densities along the line of sight. As expected, it is found that all the sources possess significantly steeper spectra below about 1 keV than observed at higher X-ray energies. Assuming a simple absorbed power-law spectral model, the mean (photon) spectral index for the sample is Gamma = 2.38 +/- 0.25, compared to the canonical 1.7 typically observed in the 2-10 keV band. Furthermore, we find strong evidence for soft X-ray spectral features in half the sources. In NGC 7469 and ESO 198-G24, we find that the addition of a narrow emission line or an absorption edge to the underlying continuum is a significant improvement to the parameterization of the spectra. Mrk 335 also shows evidence for spectral complexity, but from these data it is not possible to unambiguously distinguish between an absorption edge and a steepening of the spectrum at low energies. We examine these results in the light of the accuracy of the PSPC spectral calibration.

  11. Force Control by Flexible Manipulator Based on Resonance Ratio Control using Position Sensitive Detector

    NASA Astrophysics Data System (ADS)

    Katsura, Seiichiro; Ohnishi, Kouhei

    This paper presents a novel force controller to suppress torsional vibration of two-mass resonant system. The resonance ratio control is one of the effective control methods of two-mass resonant system. In this method, the ratio between the resonant frequency of motor and arm is determined arbitrary according to the feedback of estimated reaction torque. The reaction torque is estimated by using position sensitive detector (PSD). Since the estimation method does not need the parameter identification, the torsion information is obtained with accuracy. To attain the affinity and adaptability to environment, motion systems should control the reaction force from the environment. In the force control system, the force response is regarded as a disturbance of the arm portion. The arm disturbance is observed by the arm disturbance observer. The proposed force control system is based on both the conventional PD control and the resonance ratio control and the determination method of pole placement is discussed. The proposed force control system can realize both the suppression of the inner torsional reaction torque and the adaptation to outer force inputs. The numerical and experimental results show viability of the proposed method.

  12. A multiplexed TOF and DOI capable PET detector using a binary position sensitive network

    NASA Astrophysics Data System (ADS)

    Bieniosek, M. F.; Cates, J. W.; Levin, C. S.

    2016-11-01

    Time of flight (TOF) and depth of interaction (DOI) capabilities can significantly enhance the quality and uniformity of positron emission tomography (PET) images. Many proposed TOF/DOI PET detectors require complex readout systems using additional photosensors, active cooling, or waveform sampling. This work describes a high performance, low complexity, room temperature TOF/DOI PET module. The module uses multiplexed timing channels to significantly reduce the electronic readout complexity of the PET detector while maintaining excellent timing, energy, and position resolution. DOI was determined using a two layer light sharing scintillation crystal array with a novel binary position sensitive network. A 20 mm effective thickness LYSO crystal array with four 3 mm  ×  3 mm silicon photomultipliers (SiPM) read out by a single timing channel, one energy channel and two position channels achieved a full width half maximum (FWHM) coincidence time resolution of 180  ±  2 ps with 10 mm of DOI resolution and 11% energy resolution. With sixteen 3 mm  ×  3 mm SiPMs read out by a single timing channel, one energy channel and four position channels a coincidence time resolution 204  ±  1 ps was achieved with 10 mm of DOI resolution and 15% energy resolution. The methods presented here could significantly simplify the construction of high performance TOF/DOI PET detectors.

  13. A multiplexed TOF and DOI capable PET detector using a binary position sensitive network.

    PubMed

    Bieniosek, M F; Cates, J W; Levin, C S

    2016-11-07

    Time of flight (TOF) and depth of interaction (DOI) capabilities can significantly enhance the quality and uniformity of positron emission tomography (PET) images. Many proposed TOF/DOI PET detectors require complex readout systems using additional photosensors, active cooling, or waveform sampling. This work describes a high performance, low complexity, room temperature TOF/DOI PET module. The module uses multiplexed timing channels to significantly reduce the electronic readout complexity of the PET detector while maintaining excellent timing, energy, and position resolution. DOI was determined using a two layer light sharing scintillation crystal array with a novel binary position sensitive network. A 20 mm effective thickness LYSO crystal array with four 3 mm  ×  3 mm silicon photomultipliers (SiPM) read out by a single timing channel, one energy channel and two position channels achieved a full width half maximum (FWHM) coincidence time resolution of 180  ±  2 ps with 10 mm of DOI resolution and 11% energy resolution. With sixteen 3 mm  ×  3 mm SiPMs read out by a single timing channel, one energy channel and four position channels a coincidence time resolution 204  ±  1 ps was achieved with 10 mm of DOI resolution and 15% energy resolution. The methods presented here could significantly simplify the construction of high performance TOF/DOI PET detectors.

  14. Localized Surface Plasmon Induced Position-Sensitive Photodetection in Silicon-Nanowire-Modified Ag/Si.

    PubMed

    Mei, Chunlian; Liu, Shuai; Huang, Xu; Gan, Zhikai; Zhou, Peiqi; Wang, Hui

    2017-09-22

    Surface plasmon-based approaches are widely applied to improve the efficiency of photoelectric devices such as photosensors and photocells. In order to promote the light absorption and electron-hole pair generation in devices, metallodielectric nanostructures are used to boost the growth of surface plasmons. Here, silicon nanowires (SiNWs) are used to modify a metal-semiconductor structure; thus, Ag/SiNWs/Si is manufactured. In this system, a large increased lateral photovoltaic effect (LPE) is detected with a maximum positional sensitivity of 65.35 mV mm(-1) , which is ≈53-fold and 1000-fold compared to the conventional Ag/Si (1.24 mV mm(-1) ) and SiNWs/Si (0.06 mV mm(-1) ), respectively. It is demonstrated that localized surface plasmons (LSPs) contribute a lot to the increment of LPE. Furthermore, through the surface-enhanced Raman scattering spectra of rhodamine-6G and finite-difference time-domain simulation, it is illustrated that silver-coated SiNWs support strong LSPs. The results propose an enhancement mechanism based on LSPs to facilitate the photoelectric conversion in LPE and offer an effective way to improve the sensitivity of photodetectors. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  15. Reciprocal space mapping of epitaxial materials using position-sensitive x-ray detection

    SciTech Connect

    Lee, S.R.; Doyle, B.L.; Drummond, T.J.; Medernach, J.W.; Schneider, R.P. Jr.

    1994-10-01

    Reciprocal space mapping can be efficiently carried out using a position-sensitive x-ray detector (PSD) coupled to a traditional double-axis diffractometer. The PSD offers parallel measurement of the total scattering angle of all diffracted x-rays during a single rocking-curve scan. As a result, a two-dimensional reciprocal space map can be made in a very short time similar to that of a one-dimensional rocking-curve scan. Fast, efficient reciprocal space mapping offers numerous routine advantages to the x-ray diffraction analyst. Some of these advantages are the explicit differentiation of lattice strain from crystal orientation effects in strain-relaxed heteroepitaxial layers; the nondestructive characterization of the size, shape and orientation of nanocrystalline domains in ordered-alloy epilayers; and the ability to measure the average size and shape of voids in porous epilayers. Here, the PSD-based diffractometer is described, and specific examples clearly illustrating the advantages of complete reciprocal space analysis are presented.

  16. High spatial resolution two-dimensional position sensitive detector for the performance of coincidence experiments

    SciTech Connect

    Ceolin, D.; Chaplier, G.; Lemonnier, M.; Garcia, G.A.; Miron, C.; Nahon, L.; Simon, M.; Leclercq, N.; Morin, P.

    2005-04-01

    A position sensitive detector (PSD) adapted to the technical and mechanical specifications of our angle and energy resolved electron-ion(s) coincidence experiments is described in this article. The device, whose principle is very similar to the one detailed by J. H. D. Eland [Meas. Sci. Technol. 5, 1501 (1994)], is composed by a set of microchannel plates and a delay line anode. The originality comes from the addition in front of the encoding surface of a ceramic disk covered by a resistive surface. The capacitive coupling between the anode and the resistive plane has the double advantage of eliminating the spatial modulations due to the lattice of the anode and also of sensitizing a greater number of electrodes, increasing thus considerably the accuracy of the position measurements. The tests carried out with a time to digital conversion module of 250 ps resolution showed that a spatial resolution better than 50 {mu}m and a dead time of 160 ns can be achieved. Typical images obtained with the help of the EPICEA and DELICIOUS coincidence setups are also shown.

  17. Fourier synthesis image reconstruction by use of one-dimensional position-sensitive detectors.

    PubMed

    Kotoku, Jun'ichi; Makishima, Kazuo; Okada, Yuu; Negoro, Hitoshi; Terada, Yukikatsu; Kaneda, Hidehiro; Oda, Minoru

    2003-07-10

    An improvement of Fourier synthesis optics for hard x-ray imaging is described, and the basic performance of the new optics is confirmed through numerical simulations. The original concept of the Fourier synthesis imager utilizes nonposition-sensitive hard x-ray detectors coupled to individual bigrid modulation collimators. The improved concept employs a one-dimensional position-sensitive detector (such as a CdTe strip detector) instead of the second grid layer of each bigrid modulation collimator. This improves the imaging performance in several respects over the original design. One performance improvement is a two-fold increase in the average transmission, from 1/4 to 1/2. The second merit is that both the sine and cosine components can be derived from a single grid-detector module, and hence the number of imaging modules can be halved. Furthermore, it provides information along the depth direction simultaneously. This in turn enables a three-dimensional imaging hard x-ray microscope for medical diagnostics, incorporating radioactive tracers. A conceptual design of such a microscope is presented, designed to provide a field of view of 4 mm and a spatial resolution of 400 microm.

  18. Estimation of Compton imager using single 3D position-sensitive LYSO scintillator: Monte Carlo simulation

    NASA Astrophysics Data System (ADS)

    Lee, Taewoong; Lee, Hyounggun; Kim, Younghak; Lee, Wonho

    2017-07-01

    The performance of a Compton imager using a single three-dimensional position-sensitive LYSO scintillator detector was estimated using a Monte Carlo simulation. The Compton imager consisted of a single LYSO scintillator with a pixelized structure. The size of the scintillator and each pixel were 1.3 × 1.3 × 1.3 cm3 and 0.3 × 0.3 × 0.3 cm3, respectively. The order of γ-ray interactions was determined based on the deposited energies in each detector. After the determination of the interaction sequence, various types of reconstruction algorithms such as simple back-projection, filtered back-projection, and list-mode maximum-likelihood expectation maximization (LM-MLEM) were applied and compared with each other in terms of their angular resolution and signal-to-noise ratio (SNR) for several γ-ray energies. The LM-MLEM reconstruction algorithm exhibited the best performance for Compton imaging in maintaining high angular resolution and SNR. The two sources of 137Cs (662 keV) could be distinguishable if they were more than 17° apart. The reconstructed Compton images showed the precise position and distribution of various radiation isotopes, which demonstrated the feasibility of the monitoring of nuclear materials in homeland security and radioactive waste management applications.

  19. Single-Photon Computed Tomography With Large Position-Sensitive Phototubes*

    NASA Astrophysics Data System (ADS)

    Feldmann, John; Ranck, Amoreena; Saunders, Robert S.; Welsh, Robert E.; Bradley, Eric L.; Saha, Margaret S.; Kross, Brian; Majewski, Stan; Popov, Vladimir; Weisenberger, Andrew G.; Wojcik, Randolph

    2000-10-01

    Position-sensitive photomultiplier tubes (PSPMTs) coupled to pixelated CsI(Tl) scintillators have been used with parallel-hole collimators to view the metabolism in small animals of radiopharmaceuticals tagged with ^125I. We report here our preliminary results analyzed using a tomography program^1 written in IDL programming language. The PSPMTs are mounted on a rotating gantry so as to view the subject animal from any azimuth. Preliminary results to test the tomography algorithm have been obtained by placing a variety of plastic mouse-brain phantoms (loaded with Na^125I) in front of one of the detectors and rotating the phantom in steps through 360 degrees. Results of this simulation taken with a variety of collimator hole sizes will be compared and discussed. Extentions of this technique to the use of very small PSPMTs (Hamamatsu M-64) which are capable of a very close approach to those parts of the animal of greatest interest will be described. *Supported in part by The Department of Energy, The National Science Foundation, The American Diabetes Association, The Howard Hughes Foundation and The Jeffress Trust. 1. Tomography algorithm kindly provided by Dr. S. Meikle of The Royal Prince Albert Hospital, Sydney, Australia

  20. Position sensitive and energy dispersive x-ray detector based on silicon strip detector technology

    NASA Astrophysics Data System (ADS)

    Wiącek, P.; Dąbrowski, W.; Fink, J.; Fiutowski, T.; Krane, H.-G.; Loyer, F.; Schwamberger, A.; Świentek, K.; Venanzi, C.

    2015-04-01

    A new position sensitive detector with a global energy resolution for the entire detector of about 380 eV FWHM for 8.04 keV line at ambient temperature is presented. The measured global energy resolution is defined by the energy spectra summed over all strips of the detector, and thus it includes electronic noise of the front-end electronics, charge sharing effects, matching of parameters across the channels and other system noise sources. The target energy resolution has been achieved by segmentation of the strips to reduce their capacitance and by careful optimization of the front-end electronics. The key design aspects and parameters of the detector are discussed briefly in the paper. Excellent noise and matching performance of the readout ASIC and negligible system noise allow us to operate the detector with a discrimination threshold as low as 1 keV and to measure fluorescence radiation lines of light elements, down to Al Kα of 1.49 keV, simultaneously with measurements of the diffraction patterns. The measurement results that demonstrate the spectrometric and count rate performance of the developed detector are presented and discussed in the paper.

  1. A two-dimensional position sensitive charged-particle detector for the magnetic spectrograph ``Big Karl'' of the Jülich Cyclotron ``Jülich''

    NASA Astrophysics Data System (ADS)

    Köhler, M.; Müller, K. D.; Stoff, H.; Teske, M.; Berg, G. P. A.; Hardt, A.; Martin, S.; Mayer-Böricke, C.; Meißburger, J.

    1980-09-01

    A two-dimensional position sensitive detector with an area of 300 mm × 40 mm and a charged-particle spatial resolution of ΔX = ΔY ⩽ 0.5 mm is described. Some test results point out the detector properties. Results of the experiments 102Ru(d,p) 103Ru and 208Pb(p,p') 208Pb done at 45 MeV incident particle energy using the magnetic spectrograph BIG KARL are shown with sections of the proton spectra.

  2. Molecular Characterization of Organosulfates in Organic Aerosols from Shanghai and Los Angeles Urban Areas by Nanospray-Desorption Electrospray Ionization High-Resolution Mass Spectrometry

    SciTech Connect

    Tao, Shikang; Lu, Xiaohui; Levac, Nicole; Bateman, Adam P.; Nguyen, Tran B.; Bones, David L.; Nizkorodov, Sergey A.; Laskin, Julia; Laskin, Alexander; Yang, Xin

    2014-09-16

    Aerosol samples collected in the urban areas of Shanghai and Los Angeles were analyzed by nanospray-desorption electrospray ionization mass spectrometry (nano-DESI MS) with high mass resolution (m/Δm=100,000). Solvent mixtures of acetonitrile/water and acetonitrile/toluene were used to extract and ionize polar and non-polar compounds, respectively. A diverse mixture of oxygenated hydrocarbons, organosulfates, organonitrates, and organics with reduced nitrogen were detected in the Los Angeles sample. Majority of the organics in the Shanghai sample were detected as organosulfates. The dominant organosulfates in the two samples have distinctly different molecular characteristics. Specifically, organosulfates in the Los Angeles sample were dominated by isoprene- or monoterpene-derived products, while organosulfates of yet unknown origin in the Shanghai sample had distinctive characteristics of long aliphatic carbon chains and low degree of oxidation and unsaturation. The use of acetonitrile/toluene solvent facilitated identification of this type of organosulfates, suggesting they could be missed in previous studies relying on sample extraction using common polar solvents. The high molecular weight and low degree of unsaturation and oxidization of the organosulfates detected in the Shanghai sample suggest that they may act as surfactants, and plausibly affect the surface tension and hygroscopicity of the atmospheric particulate matter. We propose that direct esterification of carbonyl or hydroxyl compounds by sulfates or sulfuric acid in liquid phase could be the formation pathway of these special organosulfates. Finally, long-chain alkanes from vehicle emissions might be their precursors.

  3. Simultaneous data communication and position sensing with an impact ionization engineered avalanche photodiode array for free space optical communication

    NASA Astrophysics Data System (ADS)

    Ferraro, Mike S.; Mahon, Rita; Rabinovich, William S.; Murphy, James L.; Dexter, James L.; Clark, William R.; Waters, William D.; Vaccaro, Kenneth; Krejca, Brian D.

    2017-02-01

    Photodetectors in free space optical communication systems perform two functions: reception of data communication signals and position sensing for pointing, tracking, and stabilization. Traditionally, the optical receive path in an FSO system is split into separate paths for data detection and position sensing. The need for separate paths is a consequence of conflicting performance criteria between position sensitive detectors (PSD) and data detectors. Combining the functionality of both detector types requires that the combinational sensor not only have the bandwidth to support high data rate communication but the active area and spatial discrimination to accommodate position sensing. In this paper we present a large area, concentric five element impact ionization engineered avalanche photodiode array rated for bandwidths beyond 1GHz with a measured carrier ionization ratio of less than 0.1 at moderate APD gains. The integration of this array as a combinational sensor in an FSO system is discussed along with the development of a pointing and stabilization algorithm.

  4. Ionizing radiation

    USDA-ARS?s Scientific Manuscript database

    This chapter gives a comprehensive review on ionizing irradiation of fresh fruits and vegetables. Topics include principles of ionizing radiation, its effects on pathogenic and spoilage microorganisms, shelf-life, sensory quality, nutritional and phytochemical composition, as well as physiologic and...

  5. Depth of interaction resolution measurements for a high resolution PET detector using position sensitive avalanche photodiodes.

    PubMed

    Yang, Yongfeng; Dokhale, Purushottam A; Silverman, Robert W; Shah, Kanai S; McClish, Mickel A; Farrell, Richard; Entine, Gerald; Cherry, Simon R

    2006-05-07

    We explore dual-ended read out of LSO arrays with two position sensitive avalanche photodiodes (PSAPDs) as a high resolution, high efficiency depth-encoding detector for PET applications. Flood histograms, energy resolution and depth of interaction (DOI) resolution were measured for unpolished LSO arrays with individual crystal sizes of 1.0, 1.3 and 1.5 mm, and for a polished LSO array with 1.3 mm pixels. The thickness of the crystal arrays was 20 mm. Good flood histograms were obtained for all four arrays, and crystals in all four arrays can be clearly resolved. Although the amplitude of each PSAPD signal decreases as the interaction depth moves further from the PSAPD, the sum of the two PSAPD signals is essentially constant with irradiation depth for all four arrays. The energy resolutions were similar for all four arrays, ranging from 14.7% to 15.4%. A DOI resolution of 3-4 mm (including the width of the irradiation band which is approximately 2 mm) was obtained for all the unpolished arrays. The best DOI resolution was achieved with the unpolished 1 mm array (average 3.5 mm). The DOI resolution for the 1.3 mm and 1.5 mm unpolished arrays was 3.7 and 4.0 mm respectively. For the polished array, the DOI resolution was only 16.5 mm. Summing the DOI profiles across all crystals for the 1 mm array only degraded the DOI resolution from 3.5 mm to 3.9 mm, indicating that it may not be necessary to calibrate the DOI response separately for each crystal within an array. The DOI response of individual crystals in the array confirms this finding. These results provide a detailed characterization of the DOI response of these PSAPD-based PET detectors which will be important in the design and calibration of a PET scanner making use of this detector approach.

  6. Position sensitive photon detectors using epitaxial InGaAs/InAlAs quantum wells

    NASA Astrophysics Data System (ADS)

    Ganbold, T.; Antonelli, M.; Biasiol, G.; Cautero, G.; Jark, H.; Eichert, D. M.; Cucini, R.; Menk, R. H.

    2014-12-01

    This work deals with the investigation of novel position-sensitive devices based on InGaAs/InAlAs quantum wells, which could be applied to several applications of either synchrotron or conventional light sources. Such devices may be used as fast and efficient detectors due to the direct, low-energy band gap and high electron mobility at room temperature. Metamorphic In0.75Ga0.25As/In0.75Al0.25As quantum wells containing a two-dimensional electron gas were grown by molecular beam epitaxy. Two devices with size of 5 × 5 mm2 were prepared by using optical lithography. In the first, the active layers were segmented into four electrically insulated quadrants. Indium ohmic contacts were realized on the corner of each quadrant (for readout) and on the back surface (for bias). In the second, the quantum well was left unsegmented and covered by 400 nm of Al providing a single bias electrode, while four readout electrodes were fabricated on the back side by depositing and segmenting a Ni/Ge/Au layer. Photo-generated carriers can be collected at the readout electrodes by biasing from either the QW side or the back side of the devices during beam exposure. Individual currents obtained from each electrode allow monitoring of both the position and the intensity of the impinging beam for photon energies ranging from visible to hard X-ray. Such detector prototypes were tested with synchrotron radiation. Moreover, the position of the beam can be estimated with a precision of 800 nm in the segmented QW. A lower precision of 10 μm was recorded in the unsegmented QW due to the charge diffusion through the 500-μm-thick wafer, with however a lower electronic noise due to the better uniformity of the contacts.

  7. Analytical expression for position sensitivity of linear response beam position monitor having inter-electrode cross talk

    NASA Astrophysics Data System (ADS)

    Kumar, Mukesh; Ojha, A.; Garg, A. D.; Puntambekar, T. A.; Senecha, V. K.

    2017-02-01

    According to the quasi electrostatic model of linear response capacitive beam position monitor (BPM), the position sensitivity of the device depends only on the aperture of the device and it is independent of processing frequency and load impedance. In practice, however, due to the inter-electrode capacitive coupling (cross talk), the actual position sensitivity of the device decreases with increasing frequency and load impedance. We have taken into account the inter-electrode capacitance to derive and propose a new analytical expression for the position sensitivity as a function of frequency and load impedance. The sensitivity of a linear response shoe-box type BPM has been obtained through simulation using CST Studio Suite to verify and confirm the validity of the new analytical equation. Good agreement between the simulation results and the new analytical expression suggest that this method can be exploited for proper designing of BPM.

  8. Betabox: a beta particle imaging system based on a position sensitive avalanche photodiode

    PubMed Central

    Dooraghi, AA; Vu, NT; Silverman, RW; Farrell, R; Shah, KS; Wang, J; Heath, JR; Chatziioannou, AF

    2013-01-01

    A beta camera has been developed that allows planar imaging of the spatial and temporal distribution of beta particles using a 14 × 14 mm2 position sensitive avalanche photodiode (PSAPD). This camera system, which we call Betabox, can be directly coupled to microfluidic chips designed for cell incubation or other biological applications. Betabox allows for imaging the cellular uptake of molecular imaging probes labeled with charged particle emitters such as 18F inside these chips. In this work, we investigate the quantitative imaging capabilities of Betabox for 18F beta particles, in terms of background rate, efficiency, spatial resolution, and count rate. Measurements of background and spatial resolution are considered both at room temperature (21 °C ± 1 °C) and at an elevated operating temperature (37 °C ± 1 °C), as is often required for biological assays. The background rate measured with a 4 keV energy cutoff is below 2 cph mm−2 at both 21 and 37 °C. The absolute efficiency of Betabox for the detection of 18F positron sources in contact with a PSAPD with the surface passivated from ambient light and damage is 46% ± 1%. The lower detection limit is estimated using the Rose Criterion to be 0.2 cps mm−2 for 1 min acquisitions and a 62 × 62 µm2 pixel size. The upper detection limit is approximately 21 000 cps. The spatial resolution at both 21 and 37 °C ranges from 0.4 mm FWHM at the center of the field of view (FOV), and degrades to 1 mm at a distance of 5 mm away from center yielding a useful FOV of approximately 10 × 10 mm2. We also investigate the effects on spatial resolution and sensitivity that result from the use of a polymer based microfluidic chip. For these studies we place varying layers of low-density polyethylene (LDPE) between the detector and the source and find that the spatial resolution degrades by ~180 µm for every 100 µm of LDPE film. Sensitivity is reduced by half with the inclusion of ~200 µm of additional LDPE film

  9. Betabox: a beta particle imaging system based on a position sensitive avalanche photodiode

    NASA Astrophysics Data System (ADS)

    Dooraghi, A. A.; Vu, N. T.; Silverman, R. W.; Farrell, R.; Shah, K. S.; Wang, J.; Heath, J. R.; Chatziioannou, A. F.

    2013-06-01

    A beta camera has been developed that allows planar imaging of the spatial and temporal distribution of beta particles using a 14 × 14 mm2 position sensitive avalanche photodiode (PSAPD). This camera system, which we call Betabox, can be directly coupled to microfluidic chips designed for cell incubation or other biological applications. Betabox allows for imaging the cellular uptake of molecular imaging probes labeled with charged particle emitters such as 18F inside these chips. In this work, we investigate the quantitative imaging capabilities of Betabox for 18F beta particles, in terms of background rate, efficiency, spatial resolution, and count rate. Measurements of background and spatial resolution are considered both at room temperature (21 °C ± 1 °C) and at an elevated operating temperature (37 °C ± 1 °C), as is often required for biological assays. The background rate measured with a 4 keV energy cutoff is below 2 cph mm-2 at both 21 and 37 °C. The absolute efficiency of Betabox for the detection of 18F positron sources in contact with a PSAPD with the surface passivated from ambient light and damage is 46% ± 1%. The lower detection limit is estimated using the Rose Criterion to be 0.2 cps mm-2 for 1 min acquisitions and a 62 × 62 µm2 pixel size. The upper detection limit is approximately 21 000 cps. The spatial resolution at both 21 and 37 °C ranges from 0.4 mm FWHM at the center of the field of view (FOV), and degrades to 1 mm at a distance of 5 mm away from center yielding a useful FOV of approximately 10 × 10 mm2. We also investigate the effects on spatial resolution and sensitivity that result from the use of a polymer based microfluidic chip. For these studies we place varying layers of low-density polyethylene (LDPE) between the detector and the source and find that the spatial resolution degrades by ˜180 µm for every 100 µm of LDPE film. Sensitivity is reduced by half with the inclusion of ˜200 µm of additional LDPE film. Lastly

  10. New mechanism that accounts for position sensitivity of saccades evoked in response to stimulation of superior colliculus.

    PubMed

    Moschovakis, A K; Dalezios, Y; Petit, J; Grantyn, A A

    1998-12-01

    New mechanism that accounts for position sensitivity of saccades evoked in response to stimulation of superior colliculus. J. Neurophysiol. 80: 3373-3379, 1998. Electrical stimulation of the feline superior colliculus (SC) is known to evoke saccades whose size depends on the site stimulated (the "characteristic vector" of evoked saccades) and the initial position of the eyes. Similar stimuli were recently shown to produce slow drifts that are presumably caused by relatively direct projections of the SC onto extraocular motoneurons. Both slow and fast evoked eye movements are similarly affected by the initial position of the eyes, despite their dissimilar metrics, kinematics, and anatomic substrates. We tested the hypothesis that the position sensitivity of evoked saccades is due to the superposition of largely position-invariant saccades and position-dependent slow drifts. We show that such a mechanism can account for the fact that the position sensitivity of evoked saccades increases together with the size of their characteristic vector. Consistent with it, the position sensitivity of saccades drops considerably when the contribution of slow drifts is minimal as, for example, when there is no overlap between evoked saccades and short-duration trains of high-frequency stimuli.

  11. Alkali metal ionization detector

    DOEpatents

    Bauerle, James E.; Reed, William H.; Berkey, Edgar

    1978-01-01

    Variations in the conventional filament and collector electrodes of an alkali metal ionization detector, including the substitution of helical electrode configurations for either the conventional wire filament or flat plate collector; or, the substitution of a plurality of discrete filament electrodes providing an in situ capability for transferring from an operationally defective filament electrode to a previously unused filament electrode without removing the alkali metal ionization detector from the monitored environment. In particular, the helical collector arrangement which is coaxially disposed about the filament electrode, i.e. the thermal ionizer, provides an improved collection of positive ions developed by the filament electrode. The helical filament design, on the other hand, provides the advantage of an increased surface area for ionization of alkali metal-bearing species in a monitored gas environment as well as providing a relatively strong electric field for collecting the ions at the collector electrode about which the helical filament electrode is coaxially positioned. Alternatively, both the filament and collector electrodes can be helical. Furthermore, the operation of the conventional alkali metal ionization detector as a leak detector can be simplified as to cost and complexity, by operating the detector at a reduced collector potential while maintaining the sensitivity of the alkali metal ionization detector adequate for the relatively low concentration of alkali vapor and aerosol typically encountered in leak detection applications.

  12. Comparison of various stopping gases for 3He-based position sensitive neutron detectors

    NASA Astrophysics Data System (ADS)

    Doumas, A.; Smith, G. C.

    2012-05-01

    A range of solid state, scintillator and gas based detectors are being developed for use at the next generation of high flux neutron facilities. Since gas detectors are expected to continue to play a key role in future specific thermal neutron experiments, a comparison of the performance characteristics of prospective stopping gases is beneficial. Gas detectors typically utilize the reaction 3He(n,p)t to detect thermal neutrons; the 3He gas is used in a mixture containing a particular stopping gas in order to maintain relatively short ranges for the proton and triton pair emitted from the n-3He reaction. Common stopping gases include hydrocarbons (e.g. propane), carbon tetrafluoride, and noble gases such as argon and xenon. For this study, we utilized the Monte Carlo simulation code "Stopping and Range of Ions in Matter" to analyze the expected behavior of argon, xenon, carbon dioxide, difluoroethane and octafluoropropane as stopping gases for thermal neutron detectors. We also compare these findings to our previously analyzed performance of propane, butane and carbon tetrafluoride. A discussion of these gases includes their behavior in terms of proton and triton range, ionization distribution and straggle.

  13. Fast two-dimensional position-sensitive detection of neutrons in a time-of-flight reflectometer

    NASA Astrophysics Data System (ADS)

    van de Kruijs, R. W. E.; de Blois, J.

    2002-04-01

    A two-dimensional position-sensitive neutron detector with a maximum count rate of 500 kHz is described. The high counting rate is obtained by making use of dedicated electronics for data handling. The electronics convert the wire charges of a position-sensitive photomultiplier into a position using internal look-up tables. Timing modules are presented for neutron time-of-flight (TOF) determination and for dynamic measurements with an independent time-base. The position and TOF information are stored by a fast Data Handling Module. The detector is calibrated with a grid of 256×256 channels, using channel widths of 0.25 mm.The maximum error in position determination is 0.25 mm.This error is reduced to less than 0.05 mm when the electronics are used one dimensionally instead of two dimensionally. The total detector resolution was determined to be 0.6 mm.

  14. Proportional counter for X-ray analysis of lunar and planetary surfaces. [a position sensitive scintillating imaging proportional counter

    NASA Technical Reports Server (NTRS)

    1979-01-01

    A position sensitive proportional scintillation detector was developed and evaluated for use in applications involving X-ray imaging as well as spectroscopy. Topics covered include limitations of the proportional scintillation counter for use in space; purification of the xenon gas in the detector, and the operation of the detector system. Results show that the light signal in a proportional scintillation detector remains well localized. With modest electric fields in xenon, the primary electrons from a photoelectric absorption of an X-ray can be brought a distance of a few millimeters to a higher field region without spreading more than a millimeter or so. Therefore, it is possible to make a proportional scintillation detector with good position sensitivity that could be used to calibrate out the difference in light collection over its sensitive volume.

  15. Peripheral blood lymphocyte micronucleus frequencies in men from areas of Kerala, India, with high vs normal levels of natural background ionizing radiation.

    PubMed

    Karuppasamy, C V; Ramachandran, E N; Kumar, V Anil; Kumar, P R Vivek; Koya, P K M; Jaikrishan, G; Das, Birajalaxmi

    2016-04-01

    We have measured the frequencies of micronuclei (MN) in adult male individuals living in areas of the Kerala coast, southwest India, with either high (HLNRA, >1.5mGy/year) or normal levels of natural ionizing radiation (NLNRA, ≤1.5mGy/year). Blood samples were obtained from 141 individuals, 94 from HLNRA and 47 from NLNRA, aged 18-72, and were subjected to the cytokinesis-block micronucleus (CBMN) assay. An average of 1835 binucleated (BN) cells per individual were scored. The overall frequency of MN (mean±SD) was 11.7±6.7 per 1000 BN cells. The frequencies of MN in the HLNRA (11.7±6.6) and NLNRA (11.6±6.7) were not statistically significantly different (P=0.59). However, a statistically significant (P<0.001) age-dependent increase in MN frequency was observed among individuals from both HLNRA and NLNRA. No natural background radiation dose-dependent increase in MN frequency was seen. MN frequency was not influenced by tobacco smoking or chewing but it was increased among individuals consuming alcohol. Chronic low-dose radiation in the Kerala coast did not have a significant effect on MN frequency among adult men.

  16. Two-dimensional position-sensitive detectors for small-angle neutron scattering

    SciTech Connect

    McElhaney, S.A.; Vandermolen, R.I.

    1990-05-01

    In this paper, various detectors available for small angle neutron scattering (SANS) are discussed, along with some current developments being actively pursued. A section has been included to outline the various methodologies of position encoding/decoding with discussions on trends and limitations. Computer software/hardware vary greatly from institute and experiment and only a general discussion is given to this area. 85 refs., 33 figs.

  17. FUNDAMENTAL AREAS OF PHENOMENOLOGY (INCLUDING APPLICATIONS): Pulse Operation of Chemical Oxygen-Iodine Laser by Pulsed Gas Discharge with the Assistance of Spark Pre-ionization

    NASA Astrophysics Data System (ADS)

    Li, Guo-Fu; Yu, Hai-Jun; Duo, Li-Ping; Jin, Yu-Qi; Wang, Jian; Sang, Feng-Ting; Fang, Ben-Jie; Wang, De-Zhen

    2009-11-01

    The continuous wavelength chemical oxygen-iodine laser can be turned into pulse operation mode in order to obtain high energy and high pulse power. We propose an approach to produce iodine atoms instantaneously by pulsed gas discharge with the assistance of spark pre-ionization to achieve the pulsed goal. The influence of spark pre-ionization on discharge homogeneity is discussed. Voltage-current characteristics are shown and discussed in existence of the pre-ionization capacitor and peaking capacitor. The spark pre-ionization and peaking capacitor are very helpful in obtaining a stable and homogeneous discharge. The lasing is achieved at the total pressure of 2.2-2.9kPa and single pulse energy is up to 180 mJ, the corresponding specific output energy is 1.0 J/L.

  18. Development of a high-count-rate neutron detector with position sensitivity and high efficiency

    SciTech Connect

    Nelson, R.; Sandoval, J.

    1996-10-01

    While the neutron scattering community is bombarded with hints of new technologies that may deliver detectors with high-count-rate capability, high efficiency, gamma-ray insensitivity, and high resolution across large areas, only the time-tested, gas-filled {sup 3}He and scintillation detectors are in widespread use. Future spallation sources with higher fluxes simply must exploit some of the advanced detector schemes that are as yet unproved as production systems. Technologies indicating promise as neutron detectors include pixel arrays of amorphous silicon, silicon microstrips, microstrips with gas, and new scintillation materials. This project sought to study the competing neutron detector technologies and determine which or what combination will lead to a production detector system well suited for use at a high-intensity neutron scattering source.

  19. High-resolution position-sensitive proportional counter camera for radiochromatographic imaging

    SciTech Connect

    Schuresko, D.D.; Kopp, M.K.; Harter, J.A.; Bostick, W.D.

    1988-12-01

    A high-resolution proportional counter camera for imaging two- dimensional (2-D) distributions of radionuclides is described. The camera can accommodate wet or dry samples that are separated from the counter gas volume by a 6-..mu..m Mylar membrane. Using 95% Xe-5% CO/sub 2/ gas at 3-MPa pressure and electronic collimation based upon pulse energy discrimination, the camera's performance characteristics for /sup 14/C distributions are as follows: active area--10 by 10 cm, position resolution--0.5 mm, total background--300 disintegrations per minute, and count-rate capability--10/sup 5/ disintegrations per second. With computerized data acquisition, the camera is a significant improvement in analytical instrumentation for imaging 2-D radionuclide distributions over present-day commercially available technology. (Note: This manuscript was completed in July 1983). 13 refs., 10 figs.

  20. Advanced data readout technique for Multianode Position Sensitive Photomultiplier Tube applicable in radiation imaging detectors

    NASA Astrophysics Data System (ADS)

    Popov, V.

    2011-01-01

    Most of the best performing PSPMT tubes from Hamamatsu and Burle are designed with a pad-matrix anode layout. However, for obtaining a high resolution, a small-sized anode photomultiplier tubes are preferable; these tubes may have 64, 256 or 1024 anodes per tube. If the tubes are used in array to get a larger area detector, the number of analog channels may range from hundreds to thousands. Multichannel analog readout requires special electronics ICs, ASICs etc., which are attached to multichannel DAQ system. As a result, the data file and data processing time will be increased. Therefore, this readout could not be performed in a small project. Usually, most of radiation imaging applications allow the use of analog data processing in front-end electronics, significantly reducing the number of the detector's output lines to data acquisition without reducing the image quality. The idea of pad-matrix decoupling circuit with gain correction was invented and intensively tested in JLab. Several versions of PSPMT readout electronics were produced and studied. All developments were done and optimized specifically for radiation imaging projects. They covered high resolution SPECT, high speed PET, fast neutron imaging, and single tube and multi tube array systems. This paper presents and discusses the summary of the observed results in readout electronics evaluation with different PSPMTs and radiation imaging systems, as well as the advantages and limitations of the developed approach to radiation imaging detectors readout.

  1. Ionization detection system for aerosols

    DOEpatents

    Jacobs, Martin E.

    1977-01-01

    This invention relates to an improved smoke-detection system of the ionization-chamber type. In the preferred embodiment, the system utilizes a conventional detector head comprising a measuring ionization chamber, a reference ionization chamber, and a normally non-conductive gas triode for discharging when a threshold concentration of airborne particulates is present in the measuring chamber. The improved system utilizes a measuring ionization chamber which is modified to minimize false alarms and reductions in sensitivity resulting from changes in ambient temperature. In the preferred form of the modification, an annular radiation shield is mounted about the usual radiation source provided to effect ionization in the measuring chamber. The shield is supported by a bimetallic strip which flexes in response to changes in ambient temperature, moving the shield relative to the source so as to vary the radiative area of the source in a manner offsetting temperature-induced variations in the sensitivity of the chamber.

  2. Development of Gamma-Ray Compton Imager Using Room-Temperature 3-D Position Sensitive Semiconductor Detectors

    SciTech Connect

    Zhong He; David Whe; Glenn Knoll

    2003-05-14

    During the three years of this project, two 3-dimensional position sensitive CdZnTe spectrometers were upgraded in collaboration with Johns Hopkins University Applied Physics Laboratory. A prototype Compton-scattering gamma-ray imager was assembled using the two upgraded CdZnTe detectors. The performance of both gamma-ray spectrometers were individually tested. The angular resolution and detection sensitivity of the imaging system were measured using both a point and a line-shaped 137 Cs radiation source. The measurement results are consistent with that obtained from Monte-Carlo simulations performed during the early phase of the project.

  3. Simple technique for measuring the Goos-Hänchen effect with polarization modulation and a position-sensitive detector.

    PubMed

    Gilles, Hervé; Girard, Sylvain; Hamel, Joseph

    2002-08-15

    An original approach to directly measuring the Goos-Hänchen longitudinal shift between TE and TM polarization states during a total internal reflection is introduced. The technique is based on the modulation of the polarization state of a laser by an electro-optic modulator combined with a precise measurement of the resulting spatial displacement with a position-sensitive detector. This method presents many advantages over other techniques and allows measurements at different wavelengths over a broad range for the incident angle.

  4. CVD-diamond-based position sensitive photoconductive detector for high-flux x-rays and gamma rays.

    SciTech Connect

    Shu, D.

    1999-04-19

    A position-sensitive photoconductive detector (PSPCD) using insulating-type CVD diamond as its substrate material has been developed at the Advanced Photon Source (APS). Several different configurations, including a quadrant pattern for a x-ray-transmitting beam position monitor (TBPM) and 1-D and 2-D arrays for PSPCD beam profilers, have been developed. Tests on different PSPCD devices with high-heat-flux undulator white x-ray beam, as well as with gamma-ray beams from {sup 60}Co sources have been done at the APS and National Institute of Standards and Technology (NIST). It was proven that the insulating-type CVD diamond can be used to make a hard x-ray and gamma-ray position-sensitive detector that acts as a solid-state ion chamber. These detectors are based on the photoconductivity principle. A total of eleven of these TBPMs have been installed on the APS front ends for commissioning use. The linear array PSPCD beam profiler has been routinely used for direct measurements of the undulator white beam profile. More tests with hard x-rays and gamma rays are planned for the CVD-diamond 2-D imaging PSPCD. Potential applications include a high-dose-rate beam profiler for fourth-generation synchrotrons radiation facilities, such as free-electron lasers.

  5. Characterization of multipoint diffraction strain and tilt sensor based on moire interferometer and multichannel imaging position-sensitive detector

    SciTech Connect

    Iqbal, Salman; Asundi, Anand

    2006-11-15

    A multipoint diffraction strain and tilt sensor using a multichannel imaging position-sensitive detector has been developed and characterized, with the novel feature of simultaneous measurement of strain and tilt at a large array of points. Unlike conventional interferometry based systems, this new whole-field measurement system uses principles of diffraction to directly measure strain at the desired points. The system utilizes a moire interferometer for the generation of two coherent and symmetric beams, which illuminate a high-frequency diffraction grating, bonded on the surface of the sample under test. The core of the system is a charge coupled device camera fitted with an array of microlenses, which samples the diffracted beam into an array of beamlets. The camera with lens array, which is being used as array-type multichannel position-sensitive detectors, senses the shift of the individual microspots. The deviation is then processed and the normal and shear strains are calculated at that spot along with rigid-body tilt. The combined results are graphically shown to the user as two-dimensional strain and tilt maps. Simultaneous strain measurement at more than 1300 points has been successfully obtained with the spatial resolution of better than 150 {mu}m. This novel technique has many useful features compared to other whole-field optical strain measurement techniques and is expected to be very valuable in experimental mechanics of microsystems and devices.

  6. Impact-ionization-engineered avalanche photodiode arrays for free-space optical communication

    NASA Astrophysics Data System (ADS)

    Ferraro, Mike S.; Rabinovich, William S.; Clark, William R.; Waters, William D.; Campbell, Joe C.; Mahon, Rita; Vaccaro, Kenneth; Krejca, Brian D.; D'Ambrosio, Philip

    2016-11-01

    High-sensitivity photodetectors serve two purposes in free-space optical communication: data reception and position sensing for pointing, tracking, and stabilization. Two separate detectors are traditionally utilized to perform these tasks, but recent advances in the fabrication and development of large area, low-noise avalanche photodiode (APD) arrays have enabled these devices to be used both as position-sensitive detectors and communications receivers because of the conflicting performance criteria. Combining these functionalities allows for more flexibility and simplicity in optical assembly design without sacrificing the sensitivity and bandwidth performance of smaller, single-element data receivers. Beyond eliminating the need to separate the return beam into two separate paths, these devices enable implementation of adaptive approaches to compensate for focal plane beam wander and breakup, which is often seen in highly scintillated terrestrial and maritime optical links. While the Naval Research Laboratory and Optogration, Inc. have recently demonstrated the performance of single period, InAlAs/InGaAs APD arrays as combined data reception and tracking sensors, an impact-ionization-engineered epilayer design achieves even lower carrier ionization ratios by incorporating multiple multiplication periods engineered to suppress lower ionization rate carriers while enhancing the higher ionization rate carriers of interest. This work presents a three-period I2E concentric, five-element APD array rated for bandwidths beyond 1 GHz with measured carrier ionization ratios of 0.05 to 0.1 at moderate APD gains. The epilayer design of the device will be discussed along with initial device characterization and high-speed performance measurements.

  7. Impact ionization engineered avalanche photodiode arrays for free space optical communication

    NASA Astrophysics Data System (ADS)

    Ferraro, Mike S.; Rabinovich, William S.; Clark, William R.; Waters, William D.; Campbell, Joe C.; Mahon, Rita; Vaccaro, Kenneth; Krejca, Brian D.

    2016-03-01

    High sensitivity photodetectors serve two purposes in free space optical communication: data reception and position sensing for pointing, tracking, and stabilization. Because of conflicting performance criteria, two separate detectors are traditionally utilized to perform these tasks but recent advances in the fabrication and development of large area, low noise avalanche photodiode (APD) arrays have enabled these devices to be used both as position sensitive detectors (PSD) and as communications receivers. Combining these functionalities allows for more flexibility and simplicity in optical assembly design without sacrificing the sensitivity and bandwidth performance of smaller, single element data receivers. Beyond eliminating the need to separate the return beam into two separate paths, these devices enable implementation of adaptive approaches to compensate for focal plane beam wander and breakup often seen in highly scintillated terrestrial and maritime optical links. While the Naval Research Laboratory (NRL) and Optogration Inc, have recently demonstrated the performance of single period, InAlAs/InGaAs APD arrays as combined data reception and tracking sensors, an impact ionization engineered (I2E) epilayer design achieves even lower carrier ionization ratios by incorporating multiple multiplication periods engineered to suppress lower ionization rate carriers while enhancing the higher ionization rate carriers of interest. This work presents a three period I2E concentric, five element avalanche photodiode array rated for bandwidths beyond 1GHz with measured carrier ionization ratios of 0.05-0.1 at moderate APD gains. The epilayer design of the device will be discussed along with initial device characterization and high speed performance measurements.

  8. Sealed position sensitive hard X-ray detector having large drift region for all sky camera with high angular resolution

    NASA Technical Reports Server (NTRS)

    Gorenstein, P.; Perlman, D.; Parsignault, D.; Burns, R.

    1979-01-01

    A sealed position sensitive proportional counter filled with two atmospheres of 95% xenon and 5% methane, and containing a drift region of 24 atm cm, has operated in a stable manner for many months. The detector contains G-10 frames to support the anode and cathode wires. The detector was sealed successfully by a combination of vacuum baking the G-10 frames at 150 C for two weeks followed by assembly into the detector in an environment of dry nitrogen, and the use of passive internal getters. The counter is intended for use with a circumferential cylindrical collimator. Together they provide a very broad field of view detection system with the ability to locate cosmic hard X-ray and soft gamma ray sources to an angular precision of a minute of arc. A set of instruments based on this principle have been proposed for satellites to detect and precisely locate cosmic gamma ray bursts.

  9. Improving the performance of high-resolution X-ray spectrometers with position-sensitive pixel detectors.

    PubMed

    Huotari, S; Vankó, Gy; Albergamo, F; Ponchut, C; Graafsma, H; Henriquet, C; Verbeni, R; Monaco, G

    2005-07-01

    A dispersion-compensation method to remove the cube-size effect from the resolution function of diced analyzer crystals using a position-sensitive two-dimensional pixel detector is presented. For demonstration, a resolution of 23 meV was achieved with a spectrometer based on a 1 m Rowland circle and a diced Si(555) analyzer crystal in a near-backscattering geometry, with a Bragg angle of 88.5 degrees . In this geometry the spectrometer equipped with a traditional position-insensitive detector provides a resolution of 190 meV. The dispersion-compensation method thus allows a substantial increase in the resolving power without any loss of signal intensity.

  10. Integrating 2-D position sensitive X-ray detectors with low-density alkali halide storage targets

    NASA Astrophysics Data System (ADS)

    Haubold, H.-G.; Hoheisel, W.; Hiller, P.

    1986-05-01

    For the use in scattering experiments with synchrotron radiation, integrating position sensitive X-ray detectors are discussed. These detectors store the photon number equivalent charge (PNEC) in low-density alkali halide targets. Performance tests are given for a detector which uses a Gd 2O 2S fluorescence screen for X-ray detection and the low-density KCl storage target of a television SEC vidicon tube for photon integration. Rather than directly by X-rays, this target is charged by 6 keV electrons from the image intensifier section of the vidicon. Its excellent storage capability allows measurements of extremely high-contrast, high-flux X-ray patterns with the same accuracy as achieved with any single photon detection system if the discussed readout techniques are applied.

  11. Use of a YAP:Ce matrix coupled to a position-sensitive photomultiplier for high resolution positron emission tomography

    SciTech Connect

    Del Guerra, A.; Zavattini, G. |; Notaristefani, F. de |; Di Domenico, G. |; Giganti, M.; Piffanelli, A.; Pani, R.; Turra, A.

    1996-06-01

    A new scintillation detector system has been designed for application in high resolution Positron Emission Tomography (PET). The detector is a bundle of small YAlO{sub 3}:Ce (YAP) crystals closely packed (0.2 x 0.2 x 3.0 cm{sup 3}), coupled to a position sensitive photomultiplier tube (PSPMT). The preliminary results obtained for spatial resolution, time resolution, energy resolution and efficiency of two such detectors working in coincidence are presented. These are 1.2 mm for the FWHM spatial resolution, 2.0 ns for the FWHM time resolution and 20% for the FWHM energy resolution at 511 keV. The measured efficiency is (44 {+-} 3)% with a 150 keV threshold and (20 {+-} 2)% with a 300 keV threshold.

  12. Development of a position sensitive X-ray detector for use in a light weight X-ray diffractometer

    NASA Technical Reports Server (NTRS)

    Semmler, R. A.

    1971-01-01

    A position sensitive proportional counter for use in an X-ray diffractometer is developed to permit drastic reductions in the power and weight requirements of the X-ray source and the elimination of the power, weight, and complexity of a moving slit. The final detector constructed and tested has a window spanning 138 and a free standing anode curved along an arc of 7.1 cm radius. Demonstration spectra of a quartz sample in a Debye-Sherrer geometry indicate a spatial resolution of 0.4 - 0.5 mm (0.3 - 0.4 theta). The lunar diffractometer consumed 25 watts in the X-ray generator and weighed about 20 pounds.

  13. Evaluation of the x-ray response of a position-sensitive microstrip detector with an integrated readout chip

    SciTech Connect

    Rossington, C.; Jaklevic, J.; Haber, C.; Spieler, H. ); Reid, J. . Dept. of Physics)

    1990-08-01

    The performance of an SVX silicon microstrip detector and its compatible integrated readout chip have been evaluated in response to Rh K{alpha} x-rays (average energy 20.5 keV). The energy and spatial discrimination capabilities, efficient data management and fast readout rates make it an attractive alternative to the CCD and PDA detectors now being offered for x-ray position sensitive diffraction and EXAFS work. The SVX system was designed for high energy physics applications and thus further development of the existing system is required to optimize it for use in practical x-ray experiments. For optimum energy resolution the system noise must be decreased to its previously demonstrated low levels of 2 keV FWHM at 60 keV or less, and the data handling rate of the computer must be increased. New readout chips are now available that offer the potential of better performance. 15 refs., 7 figs.

  14. Position-sensitive coincidence detection of nuclear reaction products at the Prague Van-de-Graaff accelerator

    NASA Astrophysics Data System (ADS)

    Granja, Carlos; Kraus, Vaclav; Pugatch, Valery; Kohout, Zdenek

    2017-06-01

    In low-energy nuclear reactions of astrophysical interest or fusion studies the spatial- and time-correlated detection of two and more reaction products can be a valuable tool in studies of reaction mechanisms, resolving reaction channels and measuring angular distributions of reaction products. For this purpose we constructed a configurable array of position-sensitive detectors based on the hybrid semiconductor pixel detector Timepix. Additional analog-signal electronics provide self-trigger together with extended multi-device control and synchronized readout electronics by a customized control and coincidence unit. The instrumentation, developed and used for detection of fission fragments in spontaneous and neutron induced fission as well as in charged particle detection in neutron induced reactions, is being implemented for low-energy light-ion induced nuclear reactions. Application and demonstration of the technique with two Timepix detectors on p+p elastic scattering at the Van-de-Graaff (VdG) accelerator in Prague is given.

  15. Sealed position sensitive hard X-ray detector having large drift region for all sky camera with high angular resolution

    NASA Technical Reports Server (NTRS)

    Gorenstein, P.; Perlman, D.; Parsignault, D.; Burns, R.

    1979-01-01

    A sealed position sensitive proportional counter filled with two atmospheres of 95% xenon and 5% methane, and containing a drift region of 24 atm cm, has operated in a stable manner for many months. The detector contains G-10 frames to support the anode and cathode wires. The detector was sealed successfully by a combination of vacuum baking the G-10 frames at 150 C for two weeks followed by assembly into the detector in an environment of dry nitrogen, and the use of passive internal getters. The counter is intended for use with a circumferential cylindrical collimator. Together they provide a very broad field of view detection system with the ability to locate cosmic hard X-ray and soft gamma ray sources to an angular precision of a minute of arc. A set of instruments based on this principle have been proposed for satellites to detect and precisely locate cosmic gamma ray bursts.

  16. Large area neutron detector based on Li6 ionization chamber with integrated body-moderator of high density polyethylene

    SciTech Connect

    Ianakiev, Kiril D.; Swinhoe, Martyn T.; Chung, Kiwhan; Makela, Mark F.

    2009-06-30

    A detector was developed and funded by DHS to be a lower cost alternative to 3He detectors. A 6Li foil-lined ionization chamber was prepared with fill gas at one atmosphere and pulse mode operation. The high-density polyethylene (HOPE) body serves also as a neutron moderator. All electrodes, including high voltage bias supply, are hermetically sealed within the plastic slabs.

  17. Investigation on gamma-ray position sensitivity at 662 keV in a spectroscopic 3' x 3' LaBr3:Ce scintillator

    NASA Astrophysics Data System (ADS)

    Giaz, A.; Camera, F.; Birocchi, F.; Blasi, N.; Boiano, C.; Brambilla, S.; Coelli, S.; Fiorini, C.; Marone, A.; Million, B.; Riboldi, S.; Wieland, O.

    2015-02-01

    The position sensitivity of a thick, cylindrical and continuous 3" x 3" (7.62 cm x 7.62 cm) LaBr3:Ce crystal was studied using a 1 mm collimated beam of 662 keV gamma rays from a 400 MBq intense 137Cs source and a spectroscopic photomultiplier (PMT) (HAMAMATSU R6233-100SEL). The PMT entrance window was covered by black absorber except for a small window 1 cm x 1 cm wide. A complete scan of the detector over a 0.5 cm step grid was performed for three positions of the 1 cm x 1 cm window. For each configuration the energy spectrum was measured and the peak centroid, the FWHM, the area and peak asymmetry of the 662 keV gamma transition were analyzed. The data show that, even in a 3" thick LaBr3:Ce crystal with diffusive surfaces the position of the full energy peak centroid depends on the source position. We verified that, on average, the position of the full energy peak centroids measured in the three 1 cm x 1 cm window configurations is sufficient for the correct identification of the collimated gamma source position.

  18. A CdTe position sensitive detector for a hard X- and gamma-ray wide field camera

    SciTech Connect

    Caroli, E.; Cesare, G. de; Donati, A.; Dusi, W.; Landini, G.; Stephen, J.B.; Perotti, F.

    1998-12-31

    An important region of the electromagnetic spectrum for astrophysics is the hard X- and gamma ray band between 10 keV and a few MeV, where several processes occur in a wide variety of objects and with different spatial distribution and time scales. In order to fulfill the observational requirements in this energy range and taking into account the opportunities given by small/medium size missions (e.g., on the ISS), the authors have proposed a compact, wide field camera based on a thick (1 cm) position sensitive CdTe detector (PSD). The detector is made of an array of 128x96 CdTe microspectrometers with a pixel size of 2x2 mm{sup 2}. The basic element of the PSD is the linear module that is an independent detection unit with 32 CdTe crystals and monolithic front-electronics (ASIC) supported by a thin (300 {micro}m) ceramic layer. The expected performance of the PSD over the operative energy range and some of the required ASIC functionality are presented and discussed.

  19. Fast x-ray scattering measurements on molten alumina using a 120° curved position sensitive detector

    NASA Astrophysics Data System (ADS)

    Hennet, Louis; Thiaudière, Dominique; Gailhanou, Marc; Landron, Claude; Coutures, Jean-Pierre; Price, David L.

    2002-01-01

    Fast x-ray scattering measurements on molten alumina were performed on the H10 beam line at the DCI Synchrotron of LURE (Orsay, France). A high-temperature chamber with a levitation device was coupled with the four-circle goniometer of the beam line. A 100 W CO2 laser was used to melt the sample and the temperature was measured using an optical pyrometer operating at 0.85 μm. Usually, measurements of the total structure factor S(Q) on molten materials are performed using a fixed detector scanned over an angular range. In this work, in order to reduce the total scan duration, x-ray scattered intensities were measured with a 120° position sensitive detector (INEL CPS120). We performed several measurements with different acquisition times varying from 10 s to 5 min. In 5 min it was possible to obtain a good determination of S(Q) with a usable signal up to the Q range limit (13 Å-1). The intensity was comparable with a 1 h measurement with a NaI (Tl) scintillator scanned over the 120° 2θ range. On reducing the counting time the statistics are degraded and the data are noisier, especially in the high Q region. Nevertheless, even with 10 s, the S(Q) data remain usable and give good results. Performing the Fourier transformation of S(Q), we obtain similar reliable pair-correlation functions with both 5 min and 10 s acquisition times.

  20. Ultrafast molecular dynamics of dissociative ionization in OCS probed by soft x-ray synchrotron radiation

    NASA Astrophysics Data System (ADS)

    Ramadhan, Ali; Wales, Benji; Karimi, Reza; Gauthier, Isabelle; MacDonald, Michael; Zuin, Lucia; Sanderson, Joe

    2016-11-01

    Soft x-rays (90-173 eV) from the 3rd generation Canadian Light Source have been used in conjunction with a multi coincidence time and position sensitive detection apparatus to observe the dissociative ionization of OCS. By varying the x-ray energy we can compare dynamics from direct and Auger ionization processes, and access ionization channels which result in two or three body breakup, from 2+ to 4+ ionization states. We make several new observations for the 3+ state such as kinetic energy release limited by photon energy, and using Dalitz plots we can see evidence of timescale effects between the direct and Auger ionization process for the first time. Finally, using Dalitz plots for OCS4+ we observe for the first time that breakup involving an O2+ ion can only proceed from out of equilibrium nuclear arrangement for S(2p) Auger ionization.

  1. Development of a large area InGaAs APD receiver based on an impact ionization engineered detector for free-space lasercomm applications

    NASA Astrophysics Data System (ADS)

    Burris, H. R.; Ferraro, M. S.; Freeman, W. T.; Moore, C. I.; Murphy, J. L.; Rabinovich, W. S.; Smith, W. R.; Summers, L. L.; Thomas, L. M.; Vilcheck, M. J.; Clark, W. R.; Waters, W. D.

    2012-06-01

    The U.S. Naval Research Laboratory (NRL) is developing a small size, weight and power (SWaP) free space lasercomm terminal for small unmanned airborne platforms. The terminal is based on a small gimbal developed by CloudCap Technology. A receiver with a large field of view and with sensitivity sufficient to meet the program range goals is required for this terminal. An InGaAs Avalanche Photodiode (APD) with internal structures engineered to reduce excess noise and keff in high gain applications was selected as the detector. The detector is a 350 micron diameter impact ionization engineered (I2E) APD developed by Optogration, Inc. Results of development and characterization of the receiver will be presented.

  2. Spatial distortion correction and crystal identification for MRI-compatible position-sensitive avalanche photodiode-based PET scanners.

    PubMed

    Chaudhari, Abhijit J; Joshi, Anand A; Wu, Yibao; Leahy, Richard M; Cherry, Simon R; Badawi, Ramsey D

    2009-06-01

    Position-sensitive avalanche photodiodes (PSAPDs) are gaining widespread acceptance in modern PET scanner designs, and owing to their relative insensitivity to magnetic fields, especially in those that are MRI-compatible. Flood histograms in PET scanners are used to determine the crystal of annihilation photon interaction and hence, for detector characterization and routine quality control. For PET detectors that use PSAPDs, flood histograms show a characteristic pincushion distortion when Anger logic is used for event positioning. A small rotation in the flood histogram is also observed when the detectors are placed in a magnetic field. We first present a general purpose automatic method for spatial distortion correction for flood histograms of PSAPD-based PET detectors when placed both inside and outside a MRI scanner. Analytical formulae derived for this scheme are based on a hybrid approach that combines desirable properties from two existing event positioning schemes. The rotation of the flood histogram due to the magnetic field is determined iteratively and is accounted for in the scheme. We then provide implementation details of a method for crystal identification we have previously proposed and evaluate it for cases when the PET detectors are both outside and in a magnetic field. In this scheme, Fourier analysis is used to generate a lower-order spatial approximation of the distortion-corrected PSAPD flood histogram, which we call the 'template'. The template is then registered to the flood histogram using a diffeomorphic iterative intensity-based warping scheme. The calculated deformation field is then applied to the segmentation of the template to obtain a segmentation of the flood histogram. A manual correction tool is also developed for exceptional cases. We present a quantitative assessment of the proposed distortion correction scheme and crystal identification method against conventional methods. Our results indicate that our proposed methods lead to

  3. Performance measurements of a depth-encoding PET detector module based on position-sensitive avalanche photodiode read-out.

    PubMed

    Dokhale, P A; Silverman, R W; Shah, K S; Grazioso, R; Farrell, R; Glodo, J; McClish, M A; Entine, G; Tran, V H; Cherry, S R

    2004-09-21

    We are developing a high-resolution, high-efficiency positron emission tomography (PET) detector module with depth of interaction (DOI) capability based on a lutetium oxyorthosilicate (LSO) scintillator array coupled at both ends to position-sensitive avalanche photodiodes (PSAPDs). In this paper we present the DOI resolution, energy resolution and timing resolution results for complete detector modules. The detector module consists of a 7 x 7 matrix of LSO scintillator crystals (1 x 1 x 20 mm3 in dimension) coupled to 8 x 8 mm2 PSAPDs at both ends. Flood histograms were acquired and used to generate crystal look-up tables. The DOI resolution was measured for individual crystals within the array by using the ratio of the signal amplitudes from the two PSAPDs on an event-by-event basis. A measure of the total scintillation light produced was obtained by summing the signal amplitudes from the two PSAPDs. This summed signal was used to measure the energy resolution. The DOI resolution was measured to be 3-4 mm FWHM irrespective of the position of the crystal within the array, or the interaction location along the length of the crystal. The total light signal and energy resolution was almost independent of the depth of interaction. The measured energy resolution averaged 14% FWHM. The coincidence timing resolution measured using a pair of identical detector modules was 4.5 ns FWHM. These results are consistent with the design goals and the performance required of a compact, high-resolution and high-efficiency PET detector module for small animal and breast imaging applications.

  4. A data acquisition system for two-dimensional position sensitive micropattern gas detectors with delay-line readout

    NASA Astrophysics Data System (ADS)

    Hanu, A. R.; Prestwich, W. V.; Byun, S. H.

    2015-04-01

    We present a data acquisition (DAQ) system for two-dimensional position sensitive micropattern gas detectors using the delay-line method for readout. The DAQ system consists of a field programmable gate array (FPGA) as the main data processor and our time-to-digital (TDC) mezzanine card for making time measurements. We developed the TDC mezzanine card around the Acam TDC-GPX ASIC and it features four independent stop channels referenced to a common start, a typical timing resolution of ~81 ps, and a 17-bit measurement range, and is compliant with the VITA 57.1 standard. For our DAQ system, we have chosen the Xilinx SP601 development kit which features a single Spartan 6 FPGA, 128 MB of DDR2 memory, and a serial USB interface for communication. Output images consist of 1024×1024 square pixels, where each pixel has a 32-bit depth and corresponds to a time difference of 162 ps relative to its neighbours. When configured for a 250 ns acquisition window, the DAQ can resolve periodic event rates up to 1.8×106 Hz without any loses and will report a maximum event rate of 6.11×105 Hz for events whose arrival times follow Poisson statistics. The integral and differential non-linearities have also been measured and are better than 0.1% and 1.5%, respectively. Unlike commercial units, our DAQ system implements the delay-line image reconstruction algorithm entirely in hardware and is particularly attractive for its modularity, low cost, ease of integration, excellent linearity, and high throughput rate.

  5. Performance improvement of small gamma camera using NaI(Tl) plate and position sensitive photo-multiplier tubes.

    PubMed

    Jeong, Myung Hwan; Choi, Yong; Chung, Yong Hyun; Song, Tae Yong; Jung, Jin Ho; Hong, Key Jo; Min, Byung Jun; Choe, Yearn Seong; Lee, Kyung-Han; Kim, Byung-Tae

    2004-11-07

    The purpose of this study was to improve the performance of a small gamma camera, utilizing a NaI(Tl) plate and a 5" position sensitive PMT. We attempted to build a NaI(Tl) plate crystal system which retained all its advantages, while at the same time integrating some of the advantages inherent in an array-type scintillation crystal system. Flood images were obtained with a lead hole mask, and position mapping was performed by detecting hole positions in the flood image. Energy calibration was performed using the energy spectra obtained from each hole position. Flood correction was performed using a uniformity correction table containing the relative efficiency of each image element. The spatial resolution was improved about 16% after correction at the centre field of view. Resolution deterioration at the outer field of view (OFOV) was considerably ameliorated, from 6.7 mm to 3.2 mm after correction. The sensitivity at the OFOV was also increased after correction, from 0.7 cps microCi(-1) to 2.0 cps microCi(-1). The correction also improved uniformity, from 5.2% to 2.1%, and linearity, from 0.5 mm to 0 mm. The results of this study indicate that the revised correction method can be employed to considerably improve the performance of a small gamma camera using a NaI(Tl) plate-type crystal. This method also provides high spatial resolution and linearity, like array-type crystals do, while retaining the specific advantages of plate-type crystals.

  6. Background Studies of a Position Sensitive CdZnTe X-ray Detector at Balloon Altitudes

    NASA Astrophysics Data System (ADS)

    Slavis, K.; Dowkontt, P.; Epstein, J.; Hink, P.; Matteson, J.; Duttweiler, F.; Huszar, G.; Leblanc, P.; Skelton, R.; Stephan, E.

    1999-04-01

    Cadmium Zinc Telluride (CZT) is a room temperature semiconductor detector well suited for high energy X-ray astronomy. As part of the High Energy X-ray Imaging Spectrometer (HEXIS) development, we flew a position sensitive CZT detector on two balloon flights using seven shielding schemes to study the background properties of the CZT detector. Passive, active and hybrid passive-active shields were used on the cross-strip detector as well as on a standard planar CZT flown along side the cross-strip CZT for comparison. The cross-strip detector utilizes our recently developed, novel electrode configuration that improves interaction localization and depth of interaction (DOI) determination. During the flight, shield pulse heights were telemetered along with event data allowing us to conduct detailed studies of shield rejection effects. Preliminary results have been presented on the effectiveness of shielding and background reduction techniques that employ the DOI, as indicated by the ratio of cathode to anode pulse height (Slavis, et. al., SPIE Proc., 3445, 169, 1998, and Slavis, et. al., AAS #193, #66.05, 1999). Preliminary analysis indicates the 40-80 keV background is 4x10(-4) (cts)/(cm(2-s-keV)) for the cross-strip CZT without applying rejection techniques other than an active-shield energy deposition veto. We present here results incorporating more sophisticated background rejection techniques such as refinements to the preliminary DOI cut, multiple-site signatures and a more detailed investigation of the dependence of shield energy deposition on background rejection. We will also present upper limits on CZT activation. This is possible because the long duration at float in 1998 permitted cycling through the shield configurations for run times separated by at least 8 hours. Based on our preliminary analysis, we are confident that CZT detectors will be desirable for future low background, hard X-ray astronomy missions.

  7. A high count rate one-dimensional position sensitive detector and a data acquisition system for time resolved X-ray scattering studies

    NASA Astrophysics Data System (ADS)

    Pernot, P.; Kahn, R.; Fourme, R.; Leboucher, P.; Million, G.; Santiard, J. C.; Charpak, G.

    1982-10-01

    A curved multiwire proportional drift chamber has been built as a general purpose instrument for X-ray scattering and X-ray diffraction experiments with synchrotron radiation. This parallax-free one-dimensional linear position sensitive detector has a parallel readout with a double hit logic. The data acquisition system, installed as a part of the D11 camera at LURE-DCI, is designed to perform time slicing and cyclic experiments; it has been used with either the fast multiwire chamber or a standard position sensitive detector with delay line readout.

  8. Spatial distortion correction and crystal identification for MRI-compatible position-sensitive avalanche photodiode-based PET scanners

    PubMed Central

    Chaudhari, Abhijit J.; Joshi, Anand A.; Wu, Yibao; Leahy, Richard M.; Cherry, Simon R.; Badawi, Ramsey D.

    2009-01-01

    Position-sensitive avalanche photodiodes (PSAPDs) are gaining widespread acceptance in modern PET scanner designs, and owing to their relative insensitivity to magnetic fields, especially in those that are MRI-compatible. Flood histograms in PET scanners are used to determine the crystal of annihilation photon interaction and hence, for detector characterization and routine quality control. For PET detectors that use PSAPDs, flood histograms show a characteristic pincushion distortion when Anger logic is used for event positioning. A small rotation in the flood histogram is also observed when the detectors are placed in a magnetic field. We first present a general purpose automatic method for spatial distortion correction for flood histograms of PSAPD-based PET detectors when placed both inside and outside a MRI scanner. Analytical formulae derived for this scheme are based on a hybrid approach that combines desirable properties from two existing event positioning schemes. The rotation of the flood histogram due to the magnetic field is determined iteratively and is accounted for in the scheme. We then provide implementation details of a method for crystal identification we have previously proposed and evaluate it for cases when the PET detectors are both outside and in a magnetic field. In this scheme, Fourier analysis is used to generate a lower-order spatial approximation of the distortion-corrected PSAPD flood histogram, which we call the ‘template’. The template is then registered to the flood histogram using a diffeomorphic iterative intensity-based warping scheme. The calculated deformation field is then applied to the segmentation of the template to obtain a segmentation of the flood histogram. A manual correction tool is also developed for exceptional cases. We present a quantitative assessment of the proposed distortion correction scheme and crystal identification method against conventional methods. Our results indicate that our proposed methods lead

  9. The SPES surface ionization source

    NASA Astrophysics Data System (ADS)

    Manzolaro, M.; D'Agostini, F.; Monetti, A.; Andrighetto, A.

    2017-09-01

    Ion sources and target systems play a crucial role in isotope separation on line facilities, determining the main characteristics of the radioactive ion beams available for experiments. In the context of the selective production of exotic species (SPES) facility, a 40 MeV, 200 μA proton beam directly impinges a uranium carbide target, generating approximately 1013 fissions per second. The radioactive isotopes produced by the 238U fissions are delivered to the 1+ ion source by means of a tubular transfer line. Here they can be ionized and subsequently accelerated toward the experimental areas. In this work, the characterization of the surface ionization source currently adopted for the SPES facility is presented, taking as a reference ionization efficiency and transversal emittance measurements. The effects of long term operation at high temperature are also illustrated and discussed.

  10. Ionization potentials of seaborgium

    SciTech Connect

    Johnson, E.; Pershina, V.; Fricke, B.

    1999-10-21

    Multiconfiguration relativistic Dirac-Fock values were calculated for the first six ionization potentials of seaborgium and of the other group 6 elements. No experimental ionization potentials are available for seaborgium. Accurate experimental values are not available for all of the other ionization potentials. Ionic radii for the 4+ through 6+ ions of seaborgium are also presented. The ionization potentials and ionic radii obtained will be used to predict some physiochemical properties of seaborgium and its compounds.

  11. Ionization Energies of Lanthanides

    ERIC Educational Resources Information Center

    Lang, Peter F.; Smith, Barry C.

    2010-01-01

    This article describes how data are used to analyze the pattern of ionization energies of the lanthanide elements. Different observed pathways of ionization between different ground states are discussed, and the effects of pairing, exchange, and orbital interactions on ionization energies of the lanthanides are evaluated. When all the above…

  12. Ionization Energies of Lanthanides

    ERIC Educational Resources Information Center

    Lang, Peter F.; Smith, Barry C.

    2010-01-01

    This article describes how data are used to analyze the pattern of ionization energies of the lanthanide elements. Different observed pathways of ionization between different ground states are discussed, and the effects of pairing, exchange, and orbital interactions on ionization energies of the lanthanides are evaluated. When all the above…

  13. Proteomic Analysis of Flax Seeds from the Chernobyl Area Suggests Involvement of Stress, Signaling, and Transcription/Translation in Response to Ionizing Radiation

    USDA-ARS?s Scientific Manuscript database

    The accident at the Chernobyl Nuclear Power Plant (CNPP) on April 26, 1986 is the most serious nuclear disaster in human history. However, while the area proximal to the CNPP remains substantially contaminated with long-lived radioisotopes including 90Sr and 137Cs, the local ecosystem has been able...

  14. Estimation of ionizing radiation impact on natural Vicia cracca populations inhabiting areas contaminated with uranium mill tailings and radium production wastes.

    PubMed

    Evseeva, T; Majstrenko, T; Geras'kin, S; Brown, J E; Belykh, E

    2009-10-01

    Industrial areas in proximity to the Vodny settlement in the Komi Republic, Russia, have been contaminated by uranium mill tailings and radium production wastes. These areas, exhibiting high activity concentrations of naturally occurring radionuclides in soils, constitute a field laboratory where the effects of combined chronic exposures to alpha-, beta- and gamma-emitting radionuclides on natural plant populations can be studied. The aim of the present work was to determine dose-effect relationships and the range of doses that cause biological effects in natural Vicia cracca L. populations inhabiting the study area. The studied plant species is native to the area and is found ubiquitously. Soil and vegetation samples were taken at a reference location and six contaminated sites characterized by distinct floodplain depositional units with different enhanced levels of naturally occurring radionuclides. A large fraction of the dose at the study sites (including the reference location) was attributable to internal irradiation and (226)Ra was found to be an important contributor to this component of dose. The relationship between the frequency of chromosome aberrations in seedlings' root tip cells and the absorbed dose was found to be quadratic. An exponential model provided the best result in describing the empirical dependence between the absorbed dose and both the germination capacity of seeds and the survival rate of sprouts of V. cracca. For V. cracca plants inhabiting areas contaminated with uranium mill tailings and radium production wastes, a weighted absorbed dose of 0.2 Gy (weighting factor for alpha particles=5) during the vegetation period could be considered to be a level below which no increase in genetic variability and decrease in reproductive capacity might be observed above background.

  15. The 10B based Jalousie neutron detector - An alternative for 3He filled position sensitive counter tubes

    NASA Astrophysics Data System (ADS)

    Henske, M.; Klein, M.; Köhli, M.; Lennert, P.; Modzel, G.; Schmidt, C. J.; Schmidt, U.

    2012-09-01

    Over the last decades 3He filled proportional counter tubes were the working horse employed to serve as neutron counters especially in cases where large area coverage was required. Today the lack of 3He demands the development of an alternative technology. Here we present a prototype neutron detector that is based on a concept with solid 10B as neutron converter and aims for large area neutron detection applications. We report on first experimental results obtained with this prototype to demonstrate the feasibility and operational readiness of our concept.

  16. Analytical instruments, ionization sources, and ionization methods

    DOEpatents

    Atkinson, David A.; Mottishaw, Paul

    2006-04-11

    Methods and apparatus for simultaneous vaporization and ionization of a sample in a spectrometer prior to introducing the sample into the drift tube of the analyzer are disclosed. The apparatus includes a vaporization/ionization source having an electrically conductive conduit configured to receive sample particulate which is conveyed to a discharge end of the conduit. Positioned proximate to the discharge end of the conduit is an electrically conductive reference device. The conduit and the reference device act as electrodes and have an electrical potential maintained between them sufficient to cause a corona effect, which will cause at least partial simultaneous ionization and vaporization of the sample particulate. The electrical potential can be maintained to establish a continuous corona, or can be held slightly below the breakdown potential such that arrival of particulate at the point of proximity of the electrodes disrupts the potential, causing arcing and the corona effect. The electrical potential can also be varied to cause periodic arcing between the electrodes such that particulate passing through the arc is simultaneously vaporized and ionized. The invention further includes a spectrometer containing the source. The invention is particularly useful for ion mobility spectrometers and atmospheric pressure ionization mass spectrometers.

  17. Investigation of transfer ionization processes in the collision of partially stripped carbon ions on Argon

    NASA Astrophysics Data System (ADS)

    Wang, Jun; Chen, Ximeng; Ding, Baowei; Fu, Hongbin; Cui, Ying; Shao, Jianxiong; Lu, Yanxia; Gao, Zhimin; Liu, Yuwen; Du, Juan; Sun, Guangzhi; Chen, Lin

    2008-07-01

    The ratios of the cross section of the transfer-ionization to the single-electron-capture of Argon induced by C q+ ( q = 1, 2, 3) ions are measured by means of position sensitive and time-of-flight techniques. Our experimental results are compared with the data of Heq+ ( q = 1, 2) - Ar of DuBois. A qualitative interpretation is presented based on the Classical-Over-Barrier Model of Bohr.

  18. Performance of a compact position-sensitive photon counting detector with image charge coupling to an air-side anode

    NASA Astrophysics Data System (ADS)

    Jagutzki, O.; Czasch, A.; Schössler, S.

    2013-05-01

    We discuss a novel micro-channel plate (MCP) photomultiplier with resistive screen (RS-PMT) as a detection device for space- and time-correlated single photon counting, illustrated by several applications. The photomultiplier tube resembles a standard image intensifier device. However, the rear phosphor screen is replaced by a ceramic "window" with resistive coating. The MCP output is transferred through the ceramic plate to the read-out electrode (on the air side) via capacity-coupling of the image charge. This design allows for an easy reconfiguration of the read-out electrode (e.g. pixel, charge-sharing, cross-strip, delay-line) without breaking the vacuum for optimizing the detector performance towards a certain task. It also eases the design and manufacturing process of such a multi-purpose photomultiplier tube. Temporal and spatial resolutions well below 100 ps and 100 microns, respectively, have been reported at event rates as high as 1 MHz, for up to 40 mm effective detection diameter. In this paper we will discuss several applications like wide-field fluorescence microscopy and dual γ/fast-neutron radiography for air cargo screening and conclude with an outlook on large-area detectors for thermal neutrons based on MCPs.

  19. Biological Effects of Ionizing Radiation

    DOE R&D Accomplishments Database

    Ingram, M.; Mason, W. B.; Whipple, G. H.; Howland, J. W.

    1952-04-07

    This report presents a review of present knowledge and concepts of the biological effects of ionizing radiations. Among the topics discussed are the physical and chemical effects of ionizing radiation on biological systems, morphological and physiological changes observed in biological systems subjected to ionizing radiations, physiological changes in the intact animal, latent changes following exposure of biological systems to ionizing radiations, factors influencing the biological response to ionizing radiation, relative effects of various ionizing radiations, and biological dosimetry.

  20. Photoneutron depth dose equivalent distributions in high-energy X-ray medical accelerators by a novel position-sensitive dosimeter.

    PubMed

    Hakimi, Amir; Sohrabi, Mehdi

    2017-04-01

    The purpose of this study was to; (1) investigate employing a novel position-sensitive mega-size polycarbonate (MSPC) dosimeter for photoneutron (PN) depth, profile and dose equivalent distributions studies in a multilayer polyethylene phantom in a Siemens ONCOR accelerator, and (2) develop depth dose equivalent distribution matrix data at different depths and positions of the phantom for patient PN dose equivalent determination and in particular for PN secondary cancer risk estimation. Position-sensitive MSPC dosimeters were successfully exposed at 9 different depths of the phantom in a 10×10cm(2) X-ray field. The dosimeters were processed in mega-size electrochemical chambers at optimum conditions. Each MSPC dosimeter was placed at a known phantom depth for PN depth dose equivalents and profiles on transverse, longitudinal and diagonal axes and isodose equivalent distribution studies in and out of the X-ray beam. PN dose equivalent distributions at any depth showed the highest value at the beam central axis and decreases as the distance increases. PN dose equivalent at any position studied in the axes has a maximum value on the phantom surface which decreases as depth increases due to flux reduction by multi-elastic scattering interactions. Extensive PN dose equivalent matrix data at different depths and positions in the phantom were determined. The position-sensitive MSPC dosimeters proved to be highly efficient for PN depth, profile and isodose equivalent distribution studies. The extensive data obtained highly assists for determining PN dose equivalent of a patient undergoing high-energy X-ray therapy and for PN secondary cancer risk estimation. Copyright © 2017 Associazione Italiana di Fisica Medica. Published by Elsevier Ltd. All rights reserved.

  1. Note: A two-dimensional position-sensitive micro-channel plate detector with a cross-connected-pixels resistive anode and integrated spectroscopy amplifiers.

    PubMed

    Yang, Liping; Liu, Junliang; Zhang, Yuezhao; Wang, Wei; Yu, Deyang; Li, Xiaoxiao; Li, Xin; Zheng, Min; Ding, Baowei; Cai, Xiaohong

    2017-08-01

    Based on the charge-division method, a compact detector system for charged particles is constructed. The system consists of a pair of micro-channel plates, a novel two-dimensional position-sensitive cross-connected-pixels resistive anode, and specially designed front-end electronics that can directly drive analog-to-digital converters. The detector is tested with an (241)Am α-source. A position resolution of better than 0.3 mm and a maximum distortion within 0.5 mm in the active dimensions of 100 mm diameter are achieved.

  2. Ionization Phenomena in Ion-Atom Collisions

    NASA Astrophysics Data System (ADS)

    Deveney, Edward Francis

    Two many-electron ion-atom collision systems are used to investigate atomic and molecular structure and collisional interactions. Electrons emitted from MeV/u C^{3+} projectile target -atom collisions were measured with a high-resolution position -sensitive electron spectrometer at Oak Ridge National Laboratory. The electrons are predominantly ionized by direct projectile -target interactions or autoionizing (AI) from doubly excited AI levels of the ion which were excited in the collision. The energy dependence of directly scattered target electrons, binary-encounter electrons (BEE), is investigated and compared with theory. AI levels of the projectile 1s to nl single electron excited series, (1s2snl) n = 2,3,4,....infty, including the series limit are identified uniquely using energy level calculations. Original Auger yield calculations using a code by Cowan were used to discover a 1/{n^3} scaling in intensities of Auger peaks in the aforementioned series. This is explained using scattering theory. A nonstatistical population of the terms in the (1s2s2l) configuration was identified and investigated as a function of the beam energy and for four different target atoms. Two electron excited configurations are identified and investigated. The angular distribution of a correlated transfer and excitation AI state is measured and compared to theory. The final scattered charge state distributions of Kr^ {n+}, n = 1, 2, 3, 4, 5, projectiles are measured following collisions with Kr targets in the Van de Graaff Laboratory here at The University of Connecticut. Average scattered charge states as high as 12 are observed. It appears that these electrons are ionized during the lifetime of the quasimolecular state but a complete picture of the ionization mechanism(s) is not known. Calculations using a statistical model of ionization, modified in several ways, are compared with the experimental results to see if it is possible to isolate whether or not the electrons originate

  3. Electron ionization of acetylene.

    PubMed

    King, Simon J; Price, Stephen D

    2007-11-07

    Relative partial ionization cross sections and precursor specific relative partial ionization cross sections for fragment ions formed by electron ionization of C2H2 have been measured using time-of-flight mass spectrometry coupled with a 2D ion-ion coincidence technique. We report data for the formation of H+, H+2, C2+, C+/C2+ 2, CH+/C2H+2, CH+2, C+2, and C2H+ relative to the formation of C2H+2, as a function of ionizing electron energy from 30-200 eV. While excellent agreement is found between our data and one set of previously published absolute partial ionization cross sections, some discrepancies exist between the results presented here and two other recent determinations of these absolute partial ionization cross sections. We attribute these differences to the loss of some translationally energetic fragment ions in these earlier studies. Our relative precursor-specific partial ionization cross sections enable us, for the first time, to quantify the contribution to the yield of each fragment ion from single, double, and triple ionization. Analysis shows that at 50 eV double ionization contributes 2% to the total ion yield, increasing to over 10% at an ionizing energy of 100 eV. From our ion-ion coincidence data, we have derived branching ratios for charge separating dissociations of the acetylene dication. Comparison of our data to recent ab initio/RRKM calculations suggest that close to the double ionization potential C2H2+2 dissociates predominantly on the ground triplet potential energy surface (3Sigma*g) with a much smaller contribution from dissociation via the lowest singlet potential energy surface (1Delta g). Measurements of the kinetic energy released in the fragmentation reactions of C2H2+2 have been used to obtain precursor state energies for the formation of product ion pairs, and are shown to be in good agreement with available experimental data and with theory.

  4. "Magic" Ionization Mass Spectrometry.

    PubMed

    Trimpin, Sarah

    2016-01-01

    The systematic study of the temperature and pressure dependence of matrix-assisted ionization (MAI) led us to the discovery of the seemingly impossible, initially explained by some reviewers as either sleight of hand or the misinterpretation by an overzealous young scientist of results reported many years before and having little utility. The “magic” that we were attempting to report was that with matrix assistance, molecules, at least as large as bovine serum albumin (66 kDa), are lifted into the gas phase as multiply charged ions simply by exposure of the matrix:analyte sample to the vacuum of a mass spectrometer. Applied heat, a laser, or voltages are not necessary to achieve charge states and ion abundances only previously observed with electrospray ionization (ESI). The fundamentals of how solid phase volatile or nonvolatile compounds are converted to gas-phase ions without added energy currently involves speculation providing a great opportunity to rethink mechanistic understanding of ionization processes used in mass spectrometry. Improved understanding of the mechanism(s) of these processes and their connection to ESI and matrix-assisted laser desorption/ionization may provide opportunities to further develop new ionization strategies for traditional and yet unforeseen applications of mass spectrometry. This Critical Insights article covers developments leading to the discovery of a seemingly magic ionization process that is simple to use, fast, sensitive, robust, and can be directly applied to surface characterization using portable or high performance mass spectrometers.

  5. "Magic" Ionization Mass Spectrometry

    NASA Astrophysics Data System (ADS)

    Trimpin, Sarah

    2016-01-01

    The systematic study of the temperature and pressure dependence of matrix-assisted ionization (MAI) led us to the discovery of the seemingly impossible, initially explained by some reviewers as either sleight of hand or the misinterpretation by an overzealous young scientist of results reported many years before and having little utility. The "magic" that we were attempting to report was that with matrix assistance, molecules, at least as large as bovine serum albumin (66 kDa), are lifted into the gas phase as multiply charged ions simply by exposure of the matrix:analyte sample to the vacuum of a mass spectrometer. Applied heat, a laser, or voltages are not necessary to achieve charge states and ion abundances only previously observed with electrospray ionization (ESI). The fundamentals of how solid phase volatile or nonvolatile compounds are converted to gas-phase ions without added energy currently involves speculation providing a great opportunity to rethink mechanistic understanding of ionization processes used in mass spectrometry. Improved understanding of the mechanism(s) of these processes and their connection to ESI and matrix-assisted laser desorption/ionization may provide opportunities to further develop new ionization strategies for traditional and yet unforeseen applications of mass spectrometry. This Critical Insights article covers developments leading to the discovery of a seemingly magic ionization process that is simple to use, fast, sensitive, robust, and can be directly applied to surface characterization using portable or high performance mass spectrometers.

  6. Count rate studies of a box-shaped PET breast imaging system comprised of position sensitive avalanche photodiodes utilizing monte carlo simulation.

    PubMed

    Foudray, Angela M K; Habte, Frezghi; Chinn, Garry; Zhang, Jin; Levin, Craig S

    2006-01-01

    We are investigating a high-sensitivity, high-resolution positron emission tomography (PET) system for clinical use in the detection, diagnosis and staging of breast cancer. Using conventional figures of merit, design parameters were evaluated for count rate performance, module dead time, and construction complexity. The detector system modeled comprises extremely thin position-sensitive avalanche photodiodes coupled to lutetium oxy-orthosilicate scintillation crystals. Previous investigations of detector geometries with Monte Carlo indicated that one of the largest impacts on sensitivity is local scintillation crystal density when considering systems having the same average scintillation crystal densities (same crystal packing fraction and system solid-angle coverage). Our results show the system has very good scatter and randoms rejection at clinical activity ranges ( approximately 200 muCi).

  7. Determination of (235)U, (239)Pu, (240)Pu, and (241)Am in a nuclear bomb particle using a position-sensitive α-γ coincidence technique.

    PubMed

    Peräjärvi, Kari A; Ihantola, Sakari; Pöllänen, Roy C; Toivonen, Harri I; Turunen, Jani A

    2011-02-15

    A nuclear bomb particle containing 1.6 ng of Pu was investigated nondestructively with a position-sensitive α detector and a broad-energy HPGe γ-ray detector. An event-mode data acquisition system was used to record the data. α-γ coincidence counting was shown to be well suited to nondestructive isotope ratio determination. Because of the very small background, the 51.6 keV γ rays of (239)Pu and the 45.2 keV γ rays of (240)Pu were identified, which enabled isotopic ratio calculations. In the present work, the (239)Pu/((239)Pu+(240)Pu) atom ratio was determined to be 0.950 ± 0.010. The uncertainties were much smaller than in the previous more conventional nondestructive studies on this particle. Obtained results are also in good agreement with the data from the destructive mass spectrometric studies obtained previously by other investigators.

  8. Sub-nanosecond multi-channel time-to-digital converter for the 2-D position-sensitive neutron detectors at TriCS and AMOR

    NASA Astrophysics Data System (ADS)

    Buehler, Ch.; Greuter, U.; Frey, G.; Zaharko, O.; Koennecke, M.; Schefer, J.; Rasmussen, P.; Schaniel, D.; Clemens, D.; Gabriel, A.; Felsche, J.; Schlumpf, N.

    We have developed an ultra-fast multi-channel time-to-digital converter (mC-TDC). The mC-TDC electronics is used to read out the delay-line-based 2-D detectors of the neutron diffractometer and reflectometer TriCS and AMOR, respectively. The high time resolution of the mC-TDC ( 145 ps) allows the conversion of the position-sensitive detector signals into accurate 2-D scattering coordinates ( 2×2 mm2). The mC-TDC also generates low-jitter time-of-flight signals and incorporates an efficient two-stage pileup-rejection mechanism. Neutron rates exceeding 100000cps can be processed.

  9. Gas-filled position-sensitive detectors of thermal neutrons at the Konstantinov Petersburg Nuclear Physics Institute of the Russian Academy of Sciences

    NASA Astrophysics Data System (ADS)

    Andreev, V. A.; Ganzha, G. A.; Ivanov, E. A.; Ilyin, D. S.; Kovalenko, S. N.; Kolkhidashvili, M. R.; Krivshich, A. G.; Nadtochy, A. V.; Runov, V. V.; Soloveĭ, V. A.; Shabanov, G. D.

    2010-05-01

    The manufacturing line for the development and fabrication of position-sensitive detectors of thermal neutrons has been organized at the Petersburg Nuclear Physics Institute of the Russian Academy of Sciences. Three detectors with sensitive regions 300 × 170 (prototype), 200 × 200, and 300 × 300 mm in size have been constructed to date. The detectors represent multiwire proportional chambers with cathode data readout to a delay line. The devices are filled with the 3He/CF4 gas mixture. These detectors are intended for modernizing the detector systems of the Vector and Membrana-2 diffractometers (VVR-M reactor, Konstantinov Petersburg Nuclear Physics Institute of the Russian Academy of Sciences, Gatchina, Russia).

  10. Note: A two-dimensional position-sensitive micro-channel plate detector with a cross-connected-pixels resistive anode and integrated spectroscopy amplifiers

    NASA Astrophysics Data System (ADS)

    Yang, Liping; Liu, Junliang; Zhang, Yuezhao; Wang, Wei; Yu, Deyang; Li, Xiaoxiao; Li, Xin; Zheng, Min; Ding, Baowei; Cai, Xiaohong

    2017-08-01

    Based on the charge-division method, a compact detector system for charged particles is constructed. The system consists of a pair of micro-channel plates, a novel two-dimensional position-sensitive cross-connected-pixels resistive anode, and specially designed front-end electronics that can directly drive analog-to-digital converters. The detector is tested with an 241Am α-source. A position resolution of better than 0.3 mm and a maximum distortion within 0.5 mm in the active dimensions of 100 mm diameter are achieved.

  11. Comparisons of LET distributions measured in low-earth orbit using tissue-equivalent proportional counters and the position-sensitive silicon-detector telescope (RRMD-III).

    PubMed

    Doke, T; Hayashi, T; Borak, T B

    2001-09-01

    Determinations of the LET distribution, phi(L), of charged particles within a spacecraft in low-Earth orbit have been made. One method used a cylindrical tissue-equivalent proportional counter (TEPC), with the assumption that for each measured event, lineal energy, y, is equal to LET and thus phi(L) = phi(y). The other was based on the direct measurement of LETs for individual particles using a charged-particle telescope consisting of position-sensitive silicon detectors called RRMD-III. There were differences of up to a factor of 10 between estimates of phi(L) using the two methods on the same mission. This caused estimates of quality factor to vary by a factor of two between the two methods.

  12. De-Li-DAQ-2D - a new data acquisition system for position-sensitive neutron detectors with delay-line readout

    NASA Astrophysics Data System (ADS)

    Levchanovskiy, F. V.; Murashkevich, S. M.

    2016-09-01

    Software for a data acquisition system of modern one- and two-dimensional position-sensitive detectors with delay-line readout, which includes a software interface to a new electronic module De-Li-DAQ-2D with a USB interface, is presented. The new system after successful tests on the stand and on several spectrometers of the IBR-2 reactor has been integrated into the software complex SONIX+ [1]. The De-Li- DAQ-2D module [2] contains an 8-channel time-code converter (TDC-GPX) with a time resolution of 80 ps, field programmable gate array (FPGA), 1 Gbyte histogram memory and high-speed interface with a fiber-optic communication line. A real count rate is no less than 106 events/s. The De-Li-DAQ-2D module is implemented in the NIM standard. The De-Li-DAQ-2D module can operate in two modes: histogram mode and list mode.

  13. Atmospheric Ionization Measurements

    NASA Astrophysics Data System (ADS)

    Slack, Thomas; Mayes, Riley

    2015-04-01

    The measurement of atmospheric ionization is a largely unexplored science that potentially holds the key to better understanding many different geophysical phenomena through this new and valuable source of data. Through the LaACES program, which is funded by NASA through the Louisiana Space Consortium, students at Loyola University New Orleans have pursued the goal of measuring high altitude ionization for nearly three years, and were the first to successfully collect ionization data at altitudes over 30,000 feet using a scientific weather balloon flown from the NASA Columbia Scientific Ballooning Facility in Palestine, TX. In order to measure atmospheric ionization, the science team uses a lightweight and highly customized sensor known as a Gerdien condenser. Among other branches of science the data is already being used for, such as the study of aerosol pollution levels in the atmosphere, the data may also be useful in meteorology and seismology. Ionization data might provide another variable with which to predict weather or seismic activity more accurately and further in advance. Thomas Slack and Riley Mayes have served as project managers for the experiment, and have extensive knowledge of the experiment from the ground up. LaSPACE Louisiana Space Consortium.

  14. Performance evaluation of a depth-of-interaction detector by use of position-sensitive PMT with a super-bialkali photocathode.

    PubMed

    Hirano, Yoshiyuki; Nitta, Munetaka; Inadama, Naoko; Nishikido, Fumihiko; Yoshida, Eiji; Murayama, Hideo; Yamaya, Taiga

    2014-01-01

    Our purpose in this work was to evaluate the performance of a 4-layer depth-of-interaction (DOI) detector composed of GSO crystals by use of a position-sensitive photomultiplier tube (PMT) with a super-bialkali photocathode (SBA) by comparing it with a standard bialkali photocathode (BA) regarding the ability to identify the scintillating crystals, energy resolution, and timing resolution. The 4-layer DOI detector was composed of a 16 × 16 array of 2.9 × 2.9 × 7.5 mm(3) GSO crystals for each layer and an 8 × 8 multi-anode array type position-sensitive PMT. The DOI was achieved by a reflector control method, and the Anger method was used for calculating interacting points. The energy resolution in full width at half-maximum (FWHM) at 511 keV energy for the top layer (the farthest from the PMT) was improved and was 12.0% for the SBA compared with the energy resolution of 12.7% for the BA. As indicators of crystal identification ability, the peak-to-valley ratio and distance-to-width ratio were calculated; the latter was defined as the average of the distance between peaks per the average of the peak width. For both metrics, improvement of several percent was obtained; for example, the peak-to-valley ratio was increased from 1.78 (BA) to 1.86 (SBA), and the distance-to-width ratio was increased from 1.47 (BA) to 1.57 (SBA). The timing resolution (FWHM) in the bottom layer was improved slightly and was 2.4 ns (SBA) compared with 2.5 ns (BA). Better performance of the DOI detector is expected by use of a super bialkali photocathode.

  15. Ambient ionization mass spectrometry

    NASA Astrophysics Data System (ADS)

    Lebedev, A. T.

    2015-07-01

    Ambient ionization mass spectrometry emerged as a new scientific discipline only about ten years ago. A considerable body of information has been reported since that time. Keeping the sensitivity, performance and informativity of classical mass spectrometry methods, the new approach made it possible to eliminate laborious sample preparation procedures and triggered the development of miniaturized instruments to work directly in the field. The review concerns the theoretical foundations and design of ambient ionization methods. Their advantages and drawbacks, as well as prospects for application in chemistry, biology, medicine, environmetal analysis, etc., are discussed. The bibliography includes 194 references.

  16. Ionization Chamber for Prompt Fission Neutron Investigations

    NASA Astrophysics Data System (ADS)

    Zeynalov, Sh.; Zeynalova, O.; Hambsch, F.-J.; Sedyshev, P.; Shvetsov, V.

    In this work we report recent achievements in design of twin back-to-back ionization chamber (TIC) for fission fragment (FF) mass and kinetic energy measurement. Correlated FF kinetic energies, their masses and the angle of FF in respect to the axes in 3D Cartesian coordinates can be determined from analysis of the heights and shapes of the pulses induced by the fission fragments on the anodes of TIC. Anodes of TIC were designed as consisting of isolated strips each having independent electronic circuitry and special multi-channel pulse processing apparatus. Mathematical formulae provided for FF angles measured in respect to the coordinate axes. It was shown how the point of fission fragments origin on the target plane may be determined using the same measured data. The last feature made the TIC a rather powerful tool for prompt fission neutron (PFN) emission investigation in event-by-event analysis of individual fission reactions from non- point fissile source. Position sensitive neutron induced fission detector for neutron-imaging applications with both thermal and low energy neutrons was found as another possible implementation of the designed TIC.

  17. Interference effects in double ionization of spatially aligned hydrogen molecules by fast highly charged ions

    SciTech Connect

    Landers, A.L.; Alnaser, A.S.; Tanis, J.A.; Wells, E.; Osipov, T.; Carnes, K.D.; Ben-Itzhak, I.; Cocke, C.L.; McGuire, J.H.

    2004-10-01

    Cross sections differential in target orientation angle were measured for 19 MeV F{sup 8+}+D{sub 2} collisions. Multihit position-sensitive detectors were used to isolate the double-ionization channel and determine a posteriori the full momentum vectors of both ejected D{sup +} fragments. A strong dependence of the double ionization cross section on the angle between the incident ion direction and the target molecular axis is observed with a {approx_equal}3.5:1 enhancement for molecules aligned perpendicular to the projectile axis. This clear asymmetry is attributed to interference effects, analogous to Young's two-slit experiment, arising from coherent contributions to the ionization from both atomic centers. The data are compared to a simple scattering model based on two center interference.

  18. Ionizing radiation and life.

    PubMed

    Dartnell, Lewis R

    2011-01-01

    Ionizing radiation is a ubiquitous feature of the Cosmos, from exogenous cosmic rays (CR) to the intrinsic mineral radioactivity of a habitable world, and its influences on the emergence and persistence of life are wide-ranging and profound. Much attention has already been focused on the deleterious effects of ionizing radiation on organisms and the complex molecules of life, but ionizing radiation also performs many crucial functions in the generation of habitable planetary environments and the origins of life. This review surveys the role of CR and mineral radioactivity in star formation, generation of biogenic elements, and the synthesis of organic molecules and driving of prebiotic chemistry. Another major theme is the multiple layers of shielding of planetary surfaces from the flux of cosmic radiation and the various effects on a biosphere of violent but rare astrophysical events such as supernovae and gamma-ray bursts. The influences of CR can also be duplicitous, such as limiting the survival of surface life on Mars while potentially supporting a subsurface biosphere in the ocean of Europa. This review highlights the common thread that ionizing radiation forms between the disparate component disciplines of astrobiology. © Mary Ann Liebert, Inc.

  19. Microchip sonic spray ionization.

    PubMed

    Pól, Jaroslav; Kauppila, Tiina J; Haapala, Markus; Saarela, Ville; Franssila, Sami; Ketola, Raimo A; Kotiaho, Tapio; Kostiainen, Risto

    2007-05-01

    The first microchip version of sonic spray ionization (SSI) as an atmospheric pressure ionization source for mass spectrometry (MS) is presented. The microchip used for SSI has recently been developed in our laboratory, and it has been used before as an atmospheric pressure chemical ionization (APCI) and atmospheric pressure photoionization (APPI) source. Now the ionization is achieved simply by applying high (sonic) speed nebulizer gas, without heat, corona discharge, or high voltage. The microchip SSI was applied to the analysis of tetra-N-butylammonium, verapamil, testosterone, angiotensin I, and ibuprofen. The limits of detection were in the range of 15 nM to 4 microM. The technique was found to be highly dependent on the position of the chip toward the mass spectrometer inlet, and on the gas and the sample solution flow rates. The microchip SSI provided dynamic linearity following a pattern similar to that used with electrospray, good quantitative repeatability (RSD=16%), and long-term signal stability.

  20. Ionizing radiation from tobacco

    SciTech Connect

    Westin, J.B.

    1987-04-24

    Accidents at nuclear power facilities seem inevitably to bring in their wake a great deal of concern on the part of both the lay and medical communities. Relatively little attention, however, is given to what may be the largest single worldwide source of effectively carcinogenic ionizing radiation: tobacco. The risk of cancer deaths from the Chernobyl disaster are tobacco smoke is discussed.

  1. Alkali ionization detector

    DOEpatents

    Hrizo, John; Bauerle, James E.; Witkowski, Robert E.

    1982-01-01

    A calibration filament containing a sodium-bearing compound is included in combination with the sensing filament and ion collector plate of a sodium ionization detector to permit periodic generation of sodium atoms for the in-situ calibration of the detector.

  2. Electronegative plasma equilibria with spatially varying ionization

    NASA Astrophysics Data System (ADS)

    Kawamura, E.; Lichtenberg, A. J.; Lieberman, M. A.

    2012-12-01

    Electronegative inductive discharges in higher pressure ranges typically exhibit strongly localized ionization near the coil structure, with decay of the electron temperature and ionization into the central discharge region. We use a two-dimensional (2D) fluid code with a chlorine feedstock gas to determine the spatial profiles of the particle densities and electron temperature in a cylindrical transformer-coupled plasma device excited by a stove-top coil on top of the plasma chamber. To compare with one-dimensional (1D) analytical models, the 2D results are area-averaged over the radius. The area-averaged ionization frequency νiz is found to decay exponentially away from the coils, allowing the ansatz of an exponentially decaying axial variation for νiz to be used in a 1D numerical model. The 1D model captures the main features of the axial variations of the area-averaged 2D fluid simulation, indicating that the main diffusion mechanisms act along the axial direction. A simple analytical global discharge model is also developed, accounting for the asymmetric density and ionization profiles. The global model gives the scalings of the ion densities and electron temperature with power and pressure. The 1D and global models are compared with the 2D fluid simulations, showing reasonable agreement.

  3. Multifunctional Carbon Fiber Ionization Mass Spectrometry.

    PubMed

    Wu, Meng-Xi; Wang, Hao-Yang; Zhang, Jun-Ting; Guo, Yin-Long

    2016-10-04

    A carbon fiber ionization (CFI) technique was developed for the mass spectrometric analysis of various organic compounds with different polarities. The design of the CFI technique was based on the good compatibility and dispersion of samples and solutions in different solvents on carbon fiber. As a fast, convenient, and versatile ionization method, CFI-MS is especially efficient for analyzing many low/nonpolar organic compounds, such as polycyclic aromatic hydrocarbons, long-chain aliphatic aldehydes, sensitive steroids, terpenoids, and organometallic compounds. Some of these compounds may not be well-analyzed by electrospray ionization or electron ionization mass spectrometry. On the basis of our experimental results, the major ion formation mechanism of CFI-MS was suggested to involve desorption in a steam-distillation-like process, and then, ionization occurred mainly via corona discharge under high voltage. CFI-MS could not only work alone but also be coupled with separation techniques. It works well when coupled with supercritical fluid chromatography (SFC) as well as in the analysis of exhaled human air. The high flexibility and versatility of CFI-MS has extended its applications in many areas, such as fast chemical screening, clinical testing, and forensic analysis.

  4. Modulated voltage metastable ionization detector

    NASA Technical Reports Server (NTRS)

    Carle, G. C.; Kojiro, D. R.; Humphrey, D. E. (Inventor)

    1985-01-01

    The output current from a metastable ionization detector (MID) is applied to a modulation voltage circuit. An adjustment is made to balance out the background current, and an output current, above background, is applied to an input of a strip chart recorder. For low level concentrations, i.e., low detected output current, the ionization potential will be at a maximum and the metastable ionization detector will operate at its most sensitive level. When the detected current from the metastable ionization detector increases above a predetermined threshold level, a voltage control circuit is activated which turns on a high voltage transistor which acts to reduce the ionization potential. The ionization potential applied to the metastable ionization detector is then varied so as to maintain the detected signal level constant. The variation in ionization potential is now related to the concentration of the constituent and a representative amplitude is applied to another input of said strip chart recorder.

  5. Developing Benchmarks for Ionizing Radiation

    NASA Astrophysics Data System (ADS)

    Talaat, E. R.; Onsager, T. G.; Posner, A.; Allen, J. E., Jr.; Christian, E. R.; Copeland, K.; Fry, D. J.; Johnston, W. R.; Kanekal, S. G.; Kozyra, J. U.; Mertens, C. J.; Minow, J. I.; Pierson, J.; Rutledge, R.; Semones, E.; Sibeck, D. G.; St Cyr, O. C.; Xapsos, M.

    2016-12-01

    Changes in the near-Earth radiation environment can affect satellite operations, astronauts in space, commercial space activities, and the radiation environment on aircraft at relevant latitudes or altitudes. Understanding the diverse effects of increased radiation is challenging, but producing ionizing radiation benchmarks will help address these effects. The following areas have been considered in addressing the near-Earth radiation environment: the Earth's trapped radiation belts, the galactic cosmic ray background, and solar energetic-particle events. The radiation benchmarks attempt to account for any change in the near-Earth radiation environment, which, under extreme cases, could present a significant risk to critical infrastructure operations or human health. The goal of these ionizing radiation benchmarks and associated confidence levels will define at least the radiation intensity as a function of time, particle type, and energy for the following event-occurrence rate and intensity level: An occurrence frequency of 1 in 100 years; and An intensity level at the theoretical maximum for the event. The benchmarks address radiation levels at all applicable altitudes and latitudes in the near-Earth environment, and all benchmarks will state the assumptions made and the associated uncertainties.

  6. Comments on ionization cooling channels

    DOE PAGES

    Neuffer, David

    2017-09-25

    Ionization cooling channels with a wide variety of characteristics and cooling properties are being developed. These channels can produce cooling performances that are largely consistent with the linear ionization cooling theory developed previously. In this study, we review ionization cooling theory, discuss its application to presently developing cooling channels, and discuss criteria for optimizing cooling.

  7. Comments on ionization cooling channels

    NASA Astrophysics Data System (ADS)

    Neuffer, D.

    2017-09-01

    Ionization cooling channels with a wide variety of characteristics and cooling properties are being developed. These channels can produce cooling performances that are largely consistent with the linear ionization cooling theory developed previously. In this paper we review ionization cooling theory, discuss its application to presently developing cooling channels, and discuss criteria for optimizing cooling.

  8. Characterization of a sub-assembly of 3D position sensitive cadmium zinc telluride detectors and electronics from a sub-millimeter resolution PET system.

    PubMed

    Abbaszadeh, Shiva; Gu, Yi; Reynolds, Paul D; Levin, Craig S

    2016-09-21

    Cadmium zinc telluride (CZT) offers key advantages for small animal positron emission tomography (PET), including high spatial and energy resolution and simple metal deposition for fabrication of very small pixel arrays. Previous studies have investigated the intrinsic spatial, energy, and timing resolution of an individual sub-millimeter resolution CZT detector. In this work we present the first characterization results of a system of these detectors. The 3D position sensitive dual-CZT detector module and readout electronics developed in our lab was scaled up to complete a significant portion of the final PET system. This sub-system was configured as two opposing detection panels containing a total of twelve [Formula: see text] mm monolithic CZT crystals for proof of concept. System-level characterization studies, including optimizing the trigger threshold of each channel's comparators, were performed. (68)Ge and (137)Cs radioactive isotopes were used to characterize the energy resolution of all 468 anode channels in the sub-system. The mean measured global 511 keV photopeak energy resolution over all anodes was found to be [Formula: see text]% FWHM after correction for photon interaction depth-dependent signal variation. The measured global time resolution was 37 ns FWHM, a parameter to be further optimized, and the intrinsic spatial resolution was 0.76 mm FWHM.

  9. Characterization of a sub-assembly of 3D position sensitive cadmium zinc telluride detectors and electronics from a sub-millimeter resolution PET system

    NASA Astrophysics Data System (ADS)

    Abbaszadeh, Shiva; Gu, Yi; Reynolds, Paul D.; Levin, Craig S.

    2016-09-01

    Cadmium zinc telluride (CZT) offers key advantages for small animal positron emission tomography (PET), including high spatial and energy resolution and simple metal deposition for fabrication of very small pixel arrays. Previous studies have investigated the intrinsic spatial, energy, and timing resolution of an individual sub-millimeter resolution CZT detector. In this work we present the first characterization results of a system of these detectors. The 3D position sensitive dual-CZT detector module and readout electronics developed in our lab was scaled up to complete a significant portion of the final PET system. This sub-system was configured as two opposing detection panels containing a total of twelve 40~\\text{mm}× 40~\\text{mm}× 5 mm monolithic CZT crystals for proof of concept. System-level characterization studies, including optimizing the trigger threshold of each channel’s comparators, were performed. 68Ge and 137Cs radioactive isotopes were used to characterize the energy resolution of all 468 anode channels in the sub-system. The mean measured global 511 keV photopeak energy resolution over all anodes was found to be 7.35+/- 1.75 % FWHM after correction for photon interaction depth-dependent signal variation. The measured global time resolution was 37 ns FWHM, a parameter to be further optimized, and the intrinsic spatial resolution was 0.76 mm FWHM.

  10. Gridded electron reversal ionizer

    NASA Technical Reports Server (NTRS)

    Chutjian, Ara (Inventor)

    1993-01-01

    A gridded electron reversal ionizer forms a three dimensional cloud of zero or near-zero energy electrons in a cavity within a filament structure surrounding a central electrode having holes through which the sample gas, at reduced pressure, enters an elongated reversal volume. The resultant negative ion stream is applied to a mass analyzer. The reduced electron and ion space-charge limitations of this configuration enhances detection sensitivity for material to be detected by electron attachment, such as narcotic and explosive vapors. Positive ions may be generated by generating electrons having a higher energy, sufficient to ionize the target gas and pulsing the grid negative to stop the electron flow and pulsing the extraction aperture positive to draw out the positive ions.

  11. Electrospray Ionization Mass Spectrometry

    SciTech Connect

    Kelly, Ryan T.; Marginean, Ioan; Tang, Keqi

    2014-06-13

    Electrospray Ionization (ESI) is a process whereby gas phase ions are created from molecules in solution. As a solution exits a narrow tube in the presence of a strong electric field, an aerosol of charged droplets are is formed that produces gas phase ions as they it desolvates. ESI-MS comprises the creation of ions by ESI and the determination of their mass to charge ratio (m/z) by MS.

  12. Hysteresis of ionization waves

    SciTech Connect

    Dinklage, A.; Bruhn, B.; Testrich, H.; Wilke, C.

    2008-06-15

    A quasi-logistic, nonlinear model for ionization wave modes is introduced. Modes are due to finite size of the discharge and current feedback. The model consists of competing coupled modes and it incorporates spatial wave amplitude saturation. The hysteresis of wave mode transitions under current variation is reproduced. Sidebands are predicted by the model and found in experimental data. The ad hoc model is equivalent to a general--so-called universal--approach from bifurcation theory.

  13. Thin-window high-efficiency position sensitive proportional counter for the vacuum flat crystal spectrometers on the Lawrence Livermore National Laboratory electron beam ion trap (abstract)

    SciTech Connect

    Brown, G. V.; Beiersdorfer, P.; Goddard, R.; Wargelin, B.; Utter, S. B.

    2001-01-01

    We have mounted 1 {mu}m thick aluminized polyimide windows onto the position sensitive proportional counters employed by the wide-band flat crystal spectrometers at the Lawrence Livermore National Laboratory electron beam ion trap experiment. The aluminized polyimide, supported by thin wires across the short axis of the window, is used to isolate the detection chamber of the proportional counters, which operate at a pressure of 760 Torr, from the vacuum chamber of the spectrometer. The windows are modified versions of those developed for the proportional counters which were used during ground calibration of the Chandra X-ray Observatory. The transmission properties of these windows are, therefore, well known. The increased transmission efficiency of the polyimide windows relative to the 4 {mu}m thick polypropylene window material previously employed by our proportional counters has extended the useful range of the spectrometer from roughly 20 to 30 Aa at energies below the carbon edge, as well as increasing detection efficiency at wavelengths beyond the carbon edge. Using an octadecyl hydrogen maleate crystal with 2d=63.5Aa, we demonstrate the increased wavelength coverage by measuring the resonance, intercombination, and forbidden lines in helium-like NVII in two different density regimes. The thin polyimide windows have also increased the efficiency of the spectrometers entire wavelength range. To demonstrate the increased efficiency we compare the FeXVII spectrum in the 15--17 Aa band measured with the 1 {mu}m aluminized polyimide windows to the 4 {mu}m aluminized polypropylene windows. The comparison shows an average increase in efficiency of {approx}40%. The polyimide windows have a significantly lower leak rate than the polypropylene windows making it possible to achieve approximately an order of magnitude lower pressure in the spectrometer vacuum chamber which reduces the gas load on the trap region.

  14. Calcium: total or ionized?

    PubMed

    Schenck, Patricia A; Chew, Dennis J

    2008-05-01

    Measurement of serum total calcium (tCa) has been relied on for assessment of calcium status, despite the fact that it is the ionized calcium (iCa) fraction that has biologic activity. Serum tCa does not accurately predict iCa status in many clinical conditions. For accurate assessment of iCa status, iCa should be directly measured. Anaerobic measurement of serum iCa under controlled conditions provides the most reliable assessment of calcium status; aerobic measurement of iCa with species-specific pH correction is highly correlated with anaerobic measurements.

  15. Chemical protection against ionizing radiation. Final report

    SciTech Connect

    Livesey, J.C.; Reed, D.J.; Adamson, L.F.

    1984-08-01

    The scientific literature on radiation-protective drugs is reviewed. Emphasis is placed on the mechanisms involved in determining the sensitivity of biological material to ionizing radiation and mechanisms of chemical radioprotection. In Section I, the types of radiation are described and the effects of ionizing radiation on biological systems are reviewed. The effects of ionizing radiation are briefly contrasted with the effects of non-ionizing radiation. Section II reviews the contributions of various natural factors which influence the inherent radiosensitivity of biological systems. Inlcuded in the list of these factors are water, oxygen, thiols, vitamins and antioxidants. Brief attention is given to the model describing competition between oxygen and natural radioprotective substances (principally, thiols) in determining the net cellular radiosensitivity. Several theories of the mechanism(s) of action of radioprotective drugs are described in Section III. These mechanisms include the production of hypoxia, detoxication of radiochemical reactive species, stabilization of the radiobiological target and the enhancement of damage repair processes. Section IV describes the current strategies for the treatment of radiation injury. Likely areas in which fruitful research might be performed are described in Section V. 495 references.

  16. Plasma Production via Field Ionization

    SciTech Connect

    O'Connell, C.L.; Barnes, C.D.; Decker, F.; Hogan, M.J.; Iverson, R.; Krejcik, P.; Siemann, R.; Walz, D.R.; Clayton, C.E.; Huang, C.; Johnson, D.K.; Joshi, C.; Lu, W.; Marsh, K.A.; Mori, W.; Zhou, M.; Deng, S.; Katsouleas, T.; Muggli, P.; Oz, E.; /Southern California U.

    2007-01-02

    Plasma production via field ionization occurs when an incoming particle beam is sufficiently dense that the electric field associated with the beam ionizes a neutral vapor or gas. Experiments conducted at the Stanford Linear Accelerator Center explore the threshold conditions necessary to induce field ionization by an electron beam in a neutral lithium vapor. By independently varying the transverse beam size, number of electrons per bunch or bunch length, the radial component of the electric field is controlled to be above or below the threshold for field ionization. Additional experiments ionized neutral xenon and neutral nitric oxide by varying the incoming beam's bunch length. A self-ionized plasma is an essential step for the viability of plasma-based accelerators for future high-energy experiments.

  17. On accelerator-based neutron sources and neutron field characterization with low energy neutron spectrometer based on position sensitive 3He counter.

    PubMed

    Murata, I; Miyamaru, H; Kato, I; Mori, Y

    2009-07-01

    The development of new neutron sources for BNCT applications, based on particle accelerators is currently underway all over the world. Though nuclear reactors were used for a long time as the only neutron source available having the requested flux levels, the accelerator-based ones have recently been investigated on the other hand due to its easy-to-use and acceptable performances. However, when using an accelerator, various secondary particles would be emitted which forms a troublesome background. Moreover, the neutrons produced have usually an energy spectrum somewhat different from the requested one and thus should be largely moderated. An additional issue to be taken into account is the patient positioning, which should be close to the neutron source, in order to take advantage of a neutron flux level high enough to limit the BNCT treatment time within 1h. This implies that, inside a relatively narrow space, neutrons should be moderated, while unnecessary secondary particles should be shielded. Considering that a background-free neutron field from an accelerator-driven neutron source dedicated to BNCT application is generally difficult to be provided, the characterization of such a neutron field will have to be clearly assessed. In the present study, a low energy neutron spectrometer has been thus designed and is now being developed to measure the accelerator-based neutron source performance. The presently proposed spectrometer is based on a (3)He proportional counter, which is 50 cm long and 5 cm in diameter, with a gas pressure of 0.5 MPa. It is quite unique that the spectrometer is set up in parallel with the incident neutron beam and a reaction depth distribution is measured by it as a position sensitive detector. Recently, a prototype detector has been developed and the signal test is now underway. In this paper, the feature of the accelerator-based neutron sources is outlined and importance of neutron field characterization is discussed. And the developed

  18. Influence of temperature and bias voltage on the performance of a high resolution PET detector built with position sensitive avalanche photodiodes

    NASA Astrophysics Data System (ADS)

    Vandenbroucke, A.; McLaughlin, T. J.; Levin, C. S.

    2012-08-01

    We evaluate the performance of an 8 × 8 array of 0.9 × 0.9 × 1 mm3 cerium doped lutetium oxyothosilicate (LSO) crystals coupled to a position sensitive avalanche photodiode (PSAPD) as a function of bias voltage and temperature. We use this detector to develop a general methodology to optimize bias voltage, temperature, and gain for PET detectors using semiconductor photodetectors. This detector module will be used in a novel high resolution positron emission tomography (PET) camera dedicated to breast imaging under construction in our lab. Due to the tight packing of many PSAPDs in the system a thermal gradient is expected across the imaging heads. Data were collected for 11 PSAPD temperatures between 5°C and 40°C using a thermo-electric (Peltier) device. At each temperature the bias voltage was varied in steps of 5 V over a 50 V range. We present three methods to predict the optimal bias voltage at every temperature: one based on optimizing the coincidence time resolution, the others based on the relative change in PSAPD gain and leakage current due to the onset of hole multiplication. Optimal gain could also be predicted based on the quality of the flood histogram. At optimal bias voltage, the energy resolution degrades as (10.5±0.1)+((0.038±0.006)/ °C·T)%. Time resolution stays constant at 2.37±0.02 ns below 15°C. Above this temperature, time resolution deteriorates as (1.67±0.06)+((0.042±0.002)/°C·T)ns. Even at high temperatures, all 64 crystal position peaks in the flood histogram are still clearly visible. The width of the peaks in the flood histogram show a quadratic degradation with temperature: (2.6±0.1)·10-2+(1.6±0.2)·10-5/(°C)2·T2. We conclude that both the quality of the flood histogram as well as the coincidence time resolution are better parameters to estimate the optimal bias voltage, than energy resolution. Optimal bias voltage is found to be dependent on the value of k, the ratio between hole and electron multiplication. We

  19. The MICE Demonstration of Ionization Cooling

    SciTech Connect

    Pasternak, J.; Blackmore, V.; Hunt, C.; Lagrange, J-B.; Long, K.; Collomb, N.; Snopok, P.

    2015-05-01

    Muon beams of low emittance provide the basis for the intense, well-characterised neutrino beams necessary to elucidate the physics of flavour at the Neutrino Factory and to provide lepton-antilepton collisions at energies of up to several TeV at the Muon Collider. The International Muon Ionization Cooling Experiment (MICE) will demonstrate ionization cooling, the technique by which it is proposed to reduce the phase-space volume occupied by the muon beam at such facilities. In an ionization cooling channel, the muon beam passes through a material (the absorber) in which it loses energy. The energy lost is then replaced using RF cavities. The combined effect of energy loss and re-acceleration is to reduce the transverse emittance of the beam (transverse cooling). A major revision of the scope of the project was carried out over the summer of 2014. The revised project plan, which has received the formal endorsement of the international MICE Project Board and the international MICE Funding Agency Committee, will deliver a demonstration of ionization cooling by September 2017. In the revised configuration a central lithium-hydride absorber provides the cooling effect. The magnetic lattice is provided by the two superconducting focus coils and acceleration is provided by two 201 MHz single-cavity modules. The phase space of the muons entering and leaving the cooling cell will be measured by two solenoidal spectrometers. All the superconducting magnets for the ionization cooling demonstration are available at the Rutherford Appleton Laboratory and the first single-cavity prototype is under test in the MuCool Test Area at Fermilab. The design of the cooling demonstration experiment will be described together with a summary of the performance of each of its components. The cooling performance of the revised configuration will also be presented.

  20. [Ionizing and non-ionizing radiation (comparative risk estimations)].

    PubMed

    Grigor'ev, Iu G

    2012-01-01

    The population has widely used mobile communication for already more than 15 years. It is important to note that the use of mobile communication has sharply changed the conditions of daily exposure of the population to EME We expose our brain daily for the first time in the entire civilization. The mobile phone is an open and uncontrollable source of electromagnetic radiation. The comparative risk estimation for the population of ionizing and non-ionizing radiation was carried out taking into account the real conditions of influence. Comparison of risks for the population of ionizing and non-ionizing radiation leads us to a conclusion that EMF RF exposure in conditions of wide use of mobile communication is potentially more harmful than ionizing radiation influence.

  1. Ionized cluster beam deposition

    NASA Technical Reports Server (NTRS)

    Kirkpatrick, A. R.

    1983-01-01

    Ionized Cluster Beam (ICB) deposition, a new technique originated by Takagi of Kyoto University in Japan, offers a number of unique capabilities for thin film metallization as well as for deposition of active semiconductor materials. ICB allows average energy per deposited atom to be controlled and involves impact kinetics which result in high diffusion energies of atoms on the growth surface. To a greater degree than in other techniques, ICB involves quantitative process parameters which can be utilized to strongly control the characteristics of films being deposited. In the ICB deposition process, material to be deposited is vaporized into a vacuum chamber from a confinement crucible at high temperature. Crucible nozzle configuration and operating temperature are such that emerging vapor undergoes supercondensation following adiabatic expansion through the nozzle.

  2. Ionizing radiation detector

    DOEpatents

    Thacker, Louis H.

    1990-01-01

    An ionizing radiation detector is provided which is based on the principle of analog electronic integration of radiation sensor currents in the sub-pico to nano ampere range between fixed voltage switching thresholds with automatic voltage reversal each time the appropriate threshold is reached. The thresholds are provided by a first NAND gate Schmitt trigger which is coupled with a second NAND gate Schmitt trigger operating in an alternate switching state from the first gate to turn either a visible or audible indicating device on and off in response to the gate switching rate which is indicative of the level of radiation being sensed. The detector can be configured as a small, personal radiation dosimeter which is simple to operate and responsive over a dynamic range of at least 0.01 to 1000 R/hr.

  3. Multiphoton ionization of Uracil

    NASA Astrophysics Data System (ADS)

    Prieto, Eladio; Martinez, Denhi; Guerrero, Alfonso; Alvarez, Ignacio; Cisneros, Carmen

    2016-05-01

    Multiphoton ionization and dissociation of Uracil using a Reflectron time of flight spectrometer was performed along with radiation from the second harmonic of a Nd:YAG laser. Uracil is one of the four nitrogen bases that belong to RNA. The last years special interest has been concentrated on the study of the effects under UV radiation in nucleic acids1 and also in the role that this molecule could have played in the origin and development of life on our planet.2 The MPI mass spectra show that the presence and intensity of the resulting ions strongly depend on the density power. The identification of the ions in the mass spectra is presented. The results are compared with those obtained in other laboratories under different experimental conditions and some of them show partial agreement.3 The present work was supported by CONACYT-Mexico Grant 165410 and DGAPA UNAM Grant IN101215 and IN102613.

  4. Amorphous silicon ionizing particle detectors

    DOEpatents

    Street, Robert A.; Mendez, Victor P.; Kaplan, Selig N.

    1988-01-01

    Amorphous silicon ionizing particle detectors having a hydrogenated amorphous silicon (a--Si:H) thin film deposited via plasma assisted chemical vapor deposition techniques are utilized to detect the presence, position and counting of high energy ionizing particles, such as electrons, x-rays, alpha particles, beta particles and gamma radiation.

  5. Amorphous silicon ionizing particle detectors

    DOEpatents

    Street, R.A.; Mendez, V.P.; Kaplan, S.N.

    1988-11-15

    Amorphous silicon ionizing particle detectors having a hydrogenated amorphous silicon (a--Si:H) thin film deposited via plasma assisted chemical vapor deposition techniques are utilized to detect the presence, position and counting of high energy ionizing particles, such as electrons, x-rays, alpha particles, beta particles and gamma radiation. 15 figs.

  6. Exploration of the Dissociative Recombination following DNA ionization to DNA+ due to ionizing radiation

    NASA Astrophysics Data System (ADS)

    Strom, Richard A.; Zimmerly, Andrew T.; Andrianarijaona, Vola M.

    2014-05-01

    It is known that ionizing radiation generates low-energy secondary electrons, which may interact with the surrounding area, including biomolecules, such as triggering DNA single strand and double strand breaks as demonstrated by Sanche and coworkers (Radiat. Res. 157, 227(2002)). The bio-effects of low-energy electrons are currently a topic of high interest. Most of the studies are dedicated to dissociative electron attachments; however, the area is still mostly unexplored and still not well understood. We are computationally investigating the effect of ionizing radiation on DNA, such as its ionization to DNA+. More specifically, we are exploring the possibility of the dissociative recombination of the temporary DNA+ with one of the low-energy secondary electrons, produced by the ionizing radiation, to be another process of DNA strand breaks. Our preliminary results, which are performed with the binaries of ORCA, will be presented. Authors wish to give special thanks to Pacific Union College Student Senate in Angwin, California, for their financial support.

  7. Desorption/ionization on silicon nanowires.

    PubMed

    Go, E P; Apon, J V; Luo, G; Saghatelian, A; Daniels, R H; Sahi, V; Dubrow, R; Cravatt, B F; Vertes, A; Siuzdak, G

    2005-03-15

    Dense arrays of single-crystal silicon nanowires (SiNWs) have been used as a platform for laser desorption/ionization mass spectrometry of small molecules, peptides, protein digests, and endogenous and xenobiotic metabolites in biofluids. Sensitivity down to the attomole level has been achieved on the nanowire surfaces by optimizing laser energy, surface chemistry, nanowire diameter, length, and growth orientation. An interesting feature of the nanowire surface is that it requires lower laser energy as compared to porous silicon and MALDI to desorb/ionize small molecules, therefore reducing background ion interference. Taking advantage of their high surface area and fluid wicking capabilities, SiNWs were used to perform chromatographic separation followed by mass analysis of the separated molecules providing a unique platform that can integrate separation and mass spectrometric detection on a single surface.

  8. Electron-impact ionization and dissociative ionization of biomolecules

    NASA Astrophysics Data System (ADS)

    Huo, Winifred

    2006-05-01

    Oxidative damages by ionizing radiation are the source of radiation-induced damages to human health. It is recognized that secondary electrons play a role in the damage process, particularly important is the damage of DNA by electrons, potentially leading to mutagenesis. The damage can be direct, by creating a DNA lesion, or indirect, by producing radicals that attack the DNA. Molecular-level study of electron interaction with DNA provides information on the damage pathways and dominant mechanisms. This investigation focuses on ionization and dissociative ionization (DI) of DNA fragments by electron-impact. For ionization we use the improved binary-encounter dipole (iBED) model [W.M. Huo, Phys. Rev. A64, 042719-1 (2001)]. For DI it is assumed that electron motion is much faster than nuclear motion, allowing DI to be treated as a two-step process and the DI cross section given by the product of the ionization cross section and dissociation probability. The ionization study covers DNA bases, sugar phosphate backbone, and nucleotides. An additivity principle is observed. For example, the sum of the ionization cross sections of the separate deoxyribose and phosphate fragments is in close agreement with the C3'- and C5'-deoxyribose-phospate cross sections, differing by less than 5%. The result implies that certain properties of the DNA, like the total ionization cross section, are localized properties and an additivity principle may apply. This allows us to obtain properties of a larger molecular system built up from the results of smaller subsystem fragments. The DI of guanine and cytosine has been studied. For guanine, a proton is produced from the channel where the ionized electron originates from a molecular orbital with significant charge density along the N(1)-H bond. The interaction of the proton with cytosine was also studied.

  9. Electronegative Plasma Equilibria with Spatially-Varying Ionization

    NASA Astrophysics Data System (ADS)

    Lieberman, M. A.; Kawamura, E.; Lichtenberg, A. J.

    2012-10-01

    Electronegative inductive discharges in higher pressure ranges typically exhibit localized ionization near the coil structure, with decay of the ionization into the central discharge. We use a two-dimensional fluid code [1] with chlorine feedstock to determine the spatial profiles of the plasma parameters in a cylindrical transformer-coupled plasma device excited by a planar coil. To compare with one-dimensional (1D) analytic modeling, the results are area-averaged. The ionization is found to decay roughly exponentially along the axial direction, allowing the ansatz of an exponentially decaying ionization to be used in a 1D computational model. The model captures the main features of the axial variations of the area-averaged fluid simulation, indicating that the main diffusion mechanisms act along the axial direction. A simple analytic global discharge model is developed, accounting for the asymmetric density and ionization profiles. The global model gives the scalings with power and pressure of volume-averaged densities, electron temperature, and ionization decay rate, also in reasonable agreement with the scalings obtained by averaging the simulation results. [4pt] [1] E. Kawamura, D.B. Graves, and M.A. Lieberman, Plasma Sources Sci. Technol. 20, 035009 (2012)

  10. High pressure xenon ionization detector

    DOEpatents

    Markey, J.K.

    1989-11-14

    A method is provided for detecting ionization comprising allowing particles that cause ionization to contact high pressure xenon maintained at or near its critical point and measuring the amount of ionization. An apparatus is provided for detecting ionization, the apparatus comprising a vessel containing a ionizable medium, the vessel having an inlet to allow high pressure ionizable medium to enter the vessel, a means to permit particles that cause ionization of the medium to enter the vessel, an anode, a cathode, a grid and a plurality of annular field shaping rings, the field shaping rings being electrically isolated from one another, the anode, cathode, grid and field shaping rings being electrically isolated from one another in order to form an electric field between the cathode and the anode, the electric field originating at the anode and terminating at the cathode, the grid being disposed between the cathode and the anode, the field shaping rings being disposed between the cathode and the grid, the improvement comprising the medium being xenon and the vessel being maintained at a pressure of 50 to 70 atmospheres and a temperature of 0 to 30 C. 2 figs.

  11. High pressure xenon ionization detector

    DOEpatents

    Markey, John K.

    1989-01-01

    A method is provided for detecting ionization comprising allowing particles that cause ionization to contact high pressure xenon maintained at or near its critical point and measuring the amount of ionization. An apparatus is provided for detecting ionization, the apparatus comprising a vessel containing a ionizable medium, the vessel having an inlet to allow high pressure ionizable medium to enter the vessel, a means to permit particles that cause ionization of the medium to enter the vessel, an anode, a cathode, a grid and a plurality of annular field shaping rings, the field shaping rings being electrically isolated from one another, the anode, cathode, grid and field shaping rings being electrically isolated from one another in order to form an electric field between the cathode and the anode, the electric field originating at the anode and terminating at the cathode, the grid being disposed between the cathode and the anode, the field shaping rings being disposed between the cathode and the grid, the improvement comprising the medium being xenon and the vessel being maintained at a pressure of 50 to 70 atmospheres and a temperature of 0.degree. to 30.degree. C.

  12. Iron ionization and recombination rates and ionization equilibrium

    NASA Technical Reports Server (NTRS)

    Arnaud, M.; Raymond, J.

    1992-01-01

    In the past few years important progress has been made on the knowledge of ionization and recombination rates of iron, an astrophysically abundant heavy element and a major impurity in laboratory fusion devices. We make a critical review of the existing data on ionization and dielectronic recombination and present new computations of radiative recombination rate coefficients of Fe(+14) through Fe(+25) using the photoionization cross sections of Clark et al. (1986). We provide analytical fits to the recommended data (direct ionization and excitation-autoionization cross sections; radiative and dielectronic recombination rate coefficients). Finally we determine the iron ionic fractions at ionization equilibrium and compare them with previous computations as well as with observational data.

  13. Iron ionization and recombination rates and ionization equilibrium

    NASA Technical Reports Server (NTRS)

    Arnaud, M.; Raymond, J.

    1992-01-01

    In the past few years important progress has been made on the knowledge of ionization and recombination rates of iron, an astrophysically abundant heavy element and a major impurity in laboratory fusion devices. We make a critical review of the existing data on ionization and dielectronic recombination and present new computations of radiative recombination rate coefficients of Fe(+14) through Fe(+25) using the photoionization cross sections of Clark et al. (1986). We provide analytical fits to the recommended data (direct ionization and excitation-autoionization cross sections; radiative and dielectronic recombination rate coefficients). Finally we determine the iron ionic fractions at ionization equilibrium and compare them with previous computations as well as with observational data.

  14. Ionizing radiation promotes protozoan reproduction

    SciTech Connect

    Luckey, T.D.

    1986-11-01

    This experiment was performed to determine whether ionizing radiation is essential for maximum growth rate in a ciliated protozoan. When extraneous ionizing radiation was reduced to 0.15 mrad/day, the reproduction rate of Tetrahymena pyriformis was significantly less (P less than 0.01) than it was at near ambient levels, 0.5 or 1.8 mrad/day. Significantly higher growth rates (P less than 0.01) were obtained when chronic radiation was increased. The data suggest that ionizing radiation is essential for optimum reproduction rate in this organism.

  15. Pulsed helium ionization detection system

    DOEpatents

    Ramsey, R.S.; Todd, R.A.

    1985-04-09

    A helium ionization detection system is provided which produces stable operation of a conventional helium ionization detector while providing improved sensitivity and linearity. Stability is improved by applying pulsed dc supply voltage across the ionization detector, thereby modifying the sampling of the detectors output current. A unique pulse generator is used to supply pulsed dc to the detector which has variable width and interval adjust features that allows up to 500 V to be applied in pulse widths ranging from about 150 nsec to about dc conditions.

  16. Pulsed helium ionization detection system

    DOEpatents

    Ramsey, Roswitha S.; Todd, Richard A.

    1987-01-01

    A helium ionization detection system is provided which produces stable operation of a conventional helium ionization detector while providing improved sensitivity and linearity. Stability is improved by applying pulsed dc supply voltage across the ionization detector, thereby modifying the sampling of the detectors output current. A unique pulse generator is used to supply pulsed dc to the detector which has variable width and interval adjust features that allows up to 500 V to be applied in pulse widths ranging from about 150 nsec to about dc conditions.

  17. Microwave reflectometer ionization sensor

    NASA Technical Reports Server (NTRS)

    Seals, Joseph; Fordham, Jeffrey A.; Pauley, Robert G.; Simonutti, Mario D.

    1993-01-01

    The development of the Microwave Reflectometer Ionization Sensor (MRIS) Instrument for use on the Aeroassist Flight Experiment (AFE) spacecraft is described. The instrument contract was terminated, due to cancellation of the AFE program, subsequent to testing of an engineering development model. The MRIS, a four-frequency reflectometer, was designed for the detection and location of critical electron density levels in spacecraft reentry plasmas. The instrument would sample the relative magnitude and phase of reflected signals at discrete frequency steps across 4 GHz bandwidths centered at four frequencies: 20, 44, 95, and 140 GHz. The sampled data would be stored for later processing to calculate the distance from the spacecraft surface to the critical electron densities versus time. Four stepped PM CW transmitter receivers were located behind the thermal protection system of the spacecraft with horn antennas radiating and receiving through an insulating tile. Techniques were developed to deal with interference, including multiple reflections and resonance effects, resulting from the antenna configuration and operating environment.

  18. Optical ionization detector

    DOEpatents

    Wuest, Craig R.; Lowry, Mark E.

    1994-01-01

    An optical ionization detector wherein a beam of light is split so that one arm passes through a fiber optics and the other arm passes through a gas-filled region, and uses interferometry to detect density changes in a gas when charged particles pass through it. The gas-filled region of the detector is subjected to a high electric field and as a charged particle traverses this gas region electrons are freed from the cathode and accelerated so as to generate an electron avalanche which is collected on the anode. The gas density is effected by the electron avalanche formation and if the index or refraction is proportional to the gas density the index will change accordingly. The detector uses this index change by modulating the one arm of the split light beam passing through the gas, with respect to the other arm that is passed through the fiber optic. Upon recombining of the beams, interference fringe changes as a function of the index change indicates the passage of charged particles through the gaseous medium.

  19. Optical ionization detector

    DOEpatents

    Wuest, C.R.; Lowry, M.E.

    1994-03-29

    An optical ionization detector wherein a beam of light is split so that one arm passes through a fiber optics and the other arm passes through a gas-filled region, and uses interferometry to detect density changes in a gas when charged particles pass through it. The gas-filled region of the detector is subjected to a high electric field and as a charged particle traverses this gas region electrons are freed from the cathode and accelerated so as to generate an electron avalanche which is collected on the anode. The gas density is effected by the electron avalanche formation and if the index or refraction is proportional to the gas density the index will change accordingly. The detector uses this index change by modulating the one arm of the split light beam passing through the gas, with respect to the other arm that is passed through the fiber optic. Upon recombining of the beams, interference fringe changes as a function of the index change indicates the passage of charged particles through the gaseous medium. 3 figures.

  20. The Ionization History of The Intergalactic Medium:

    NASA Technical Reports Server (NTRS)

    Madau, Piero

    2003-01-01

    The funded project seeked a unified description of the ionization, physical structure, and evolution of the intergalactic medium (IGM) and quasar intervening absorption systems. We proposed to conduct theoretical studies of the IGM and QSO absorbers in the context of current theories of galaxy formation, developing and using numerical and analytical techniques aimed at a detailed modeling of cosmological radiative transfer, gas dynamics, and thermal and ionization evolution. The ionization history of the IGM has important implications for the metagalactic UV background, intergalactic helium absorption 21-cm tomography, metal absorption systems, fluctuations in the microwave background, and the cosmic rate of structure and star formation. All the original objectives of our program have been achieved, and the results widely used and quoted by the community. Indeed, they remain relevant as the level and complexity of research in this area has increased substantially since our proposal was submitted, due to new discoveries on galaxy formation and evolution, a flood of high-quality data on the distant universe, new theoretical ideas and direct numerical simulations of structure formation in hierarchical clustering theories.

  1. Ionization oscillations in Hall accelerators

    NASA Astrophysics Data System (ADS)

    Barral, S.; Peradzyński, Z.

    2010-01-01

    The underlying mechanism of low-frequency oscillations in Hall accelerators is investigated theoretically. It is shown that relaxation oscillations arise from a competition between avalanche ionization and the advective transport of the working gas. The model derived recovers the slow progression and fast recession of the ionization front. Analytical approximations of the shape of current pulses and of the oscillation frequency are provided for the case of large amplitude oscillations.

  2. Resonance ionization for analytical spectroscopy

    DOEpatents

    Hurst, George S.; Payne, Marvin G.; Wagner, Edward B.

    1976-01-01

    This invention relates to a method for the sensitive and selective analysis of an atomic or molecular component of a gas. According to this method, the desired neutral component is ionized by one or more resonance photon absorptions, and the resultant ions are measured in a sensitive counter. Numerous energy pathways are described for accomplishing the ionization including the use of one or two tunable pulsed dye lasers.

  3. Zero-Net-Charge Air Ionizer

    NASA Technical Reports Server (NTRS)

    Woods, W. R., Jr.

    1985-01-01

    Instrument monitors air supplied by air ionizer and regulates ionizer to ensure net charge neutral. High-impedance electrometer and nulling control amplifier regulate output of air ionizer. Primarily intended to furnish ionized air having no net charge, instrument adaptable to generating air with positive or negative net charge is so desired. Useful where integrated circuit chips are manufactured, inspected, tested or assembled.

  4. Reduced Sampling Size with Nanopipette for Tapping-Mode Scanning Probe Electrospray Ionization Mass Spectrometry Imaging

    PubMed Central

    Kohigashi, Tsuyoshi; Otsuka, Yoichi; Shimazu, Ryo; Matsumoto, Takuya; Iwata, Futoshi; Kawasaki, Hideya; Arakawa, Ryuichi

    2016-01-01

    Mass spectrometry imaging (MSI) with ambient sampling and ionization can rapidly and easily capture the distribution of chemical components in a solid sample. Because the spatial resolution of MSI is limited by the size of the sampling area, reducing sampling size is an important goal for high resolution MSI. Here, we report the first use of a nanopipette for sampling and ionization by tapping-mode scanning probe electrospray ionization (t-SPESI). The spot size of the sampling area of a dye molecular film on a glass substrate was decreased to 6 μm on average by using a nanopipette. On the other hand, ionization efficiency increased with decreasing solvent flow rate. Our results indicate the compatibility between a reduced sampling area and the ionization efficiency using a nanopipette. MSI of micropatterns of ink on a glass and a polymer substrate were also demonstrated. PMID:28101441

  5. Single ionization of molecular iodine

    NASA Astrophysics Data System (ADS)

    Smith, Dale L.; Tagliamonti, Vincent; Dragan, James; Gibson, George N.

    2017-01-01

    We performed a study of the single ionization of iodine, I2 over a range of wavelengths. Single ionization of I2 is unexpectedly found to have a contribution from inner molecular orbitals involving the 5 s electrons. The I+I+ dissociation channel was recorded through velocity map imaging, and the kinetic-energy release of each channel was determined with two-dimensional fitting of the images. Most of the measured kinetic-energy data were inconsistent with ionization to the X , A , and B states of I2 + , implying ionization from deeper orbitals. A pump-probe Fourier transform technique was used to look for modulation at the X - and A -state vibrational frequencies to see if they were intermediate states in a two-step process. X - and A -state modulation was seen only for kinetic-energy releases below 0.2 eV, consistent with dissociation through the B state. From these results and intensity-, polarization-, and wavelength-dependent experiments we found no evidence of bond softening, electron rescattering, or photon mediation through the X or A states to higher-energy single-ionization channels.

  6. Ionizing radiation injuries and illnesses.

    PubMed

    Christensen, Doran M; Iddins, Carol J; Sugarman, Stephen L

    2014-02-01

    Although the spectrum of information related to diagnosis and management of radiation injuries and illnesses is vast and as radiation contamination incidents are rare, most emergency practitioners have had little to no practical experience with such cases. Exposures to ionizing radiation and internal contamination with radioactive materials can cause significant tissue damage and conditions. Emergency practitioners unaware of ionizing radiation as the cause of a condition may miss the diagnosis of radiation-induced injury or illness. This article reviews the pertinent terms, physics, radiobiology, and medical management of radiation injuries and illnesses that may confront the emergency practitioner. Copyright © 2014 Elsevier Inc. All rights reserved.

  7. Breakup of loosely bound nuclei at intermediate energies for nuclear astrophysics and the development of a position sensitive microstrip detector system and its readout electronics using ASICs technologies

    SciTech Connect

    Bertulani, Carlos A.

    2016-01-12

    The work performed under this grant has led to the development of a detection system that will be used to measure reaction rates for proton or neutron capture reactions at stellar energies on radioactive ions far from stability. The reaction rates are needed to better understand the physics of nucleosynthesis in explosive stellar processes such as supernovae and x-ray burst events. The radioactive ions will be produced at the Radioactive Ion Beam Facility (RIBF) at RIKEN near Tokyo, Japan. During the course of this work, the group involved in this project has expanded by several institutions in Europe and Japan and now involves collaborators from the U.S., Japan, Hungary, Romania, Germany, Spain, Italy, China, and South Korea. As part of the project, a novel design based on large-area silicon detectors has been built and tested. The work has involved mechanical construction of a special purpose vacuum chamber, with a precision mounting system for the silicon detectors, development of a new ASICs readout system that has applications with a wide variety of silicon detector systems, and the development of a data acquisition system that is integrated into the computer system being used at RIBF. The parts noted above that are needed to carry out the research program are completed and ready for installation. Several approved experiments that will use this system will be carried out in the near future. The experimental work has been delayed due to a large increase in the cost and availability of electrical power for RIBF that occurred following the massive earthquake and tsunami that hit Japan in the spring of 2011. Another component of the research carried out with this grant involved developing the theoretical tools that are required to extract the information from the experiments that is needed to determine the stellar reaction rates. The tools developed through this part of the work will be made freely available for general use.

  8. (Workshop on artificially ionized layers in the atmosphere)

    SciTech Connect

    Tunnell, T.W.

    1989-10-30

    I presented our report which described our technique of inferring electron temperature in a microwave induced plasma. The primary purpose of my trip to Kiev was to present a paper entitled Analysis of Nitrogen Light Emission from Artificially Ionized Layers (AIL) Breakdown'' at the AIL workshop. The AIL concept is to produce an ionized layer in the atmosphere from which radio frequency waves can be reflected. The workshop provided for the transfer of unclassified technology between the US and the USSR, who are reportedly years, if not decades, ahead of the US in this area of research.

  9. Breakup of loosely bound nuclei at intermediate energies for nuclear astrophysics and the development of a position sensitive microstrip detector system and its readout electronics using ASICs technologies

    SciTech Connect

    Tribble, Robert E.; Sobotka, Lee G.; Blackmon, Jeff C.; Bertulani, Carlos A.

    2015-12-29

    The work performed under this grant has led to the development of a detection system that will be used to measure reaction rates for proton or neutron capture reactions at stellar energies on radioactive ions far from stability. The reaction rates are needed to better understand the physics of nucleosynthesis in explosive stellar processes such as supernovae and x-ray burst events. The radioactive ions will be produced at the Radioactive Ion Beam Facility (RIBF) at RIKEN near Tokyo, Japan. During the course of this work, the group involved in this project has expanded by several institutions in Europe and Japan and now involves collaborators from the U.S., Japan, Hungary, Romania, Germany, Spain, Italy, China, and South Korea. As part of the project, a novel design based on large-area silicon detectors has been built and tested and the performance characterized in a series of tests using particle beams with a variety of atomic numbers at the Cyclotron Institute of Texas A&M University and the Heavy Ion Medical Accelerator in Chiba facility (HIMAC) in Chiba, Japan. The work has involved mechanical construction of a special purpose vacuum chamber, with a precision mounting system for the silicon detectors, development of a new ASICs readout system that has applications with a wide variety of silicon detector systems, and the development of a data acquisition system that is integrated into the computer system being used at RIBF. The parts noted above that are needed to carry out the research program are completed and ready for installation. Several approved experiments that will use this system will be carried out in the near future. The experimental work has been delayed due to a large increase in the cost and availability of electrical power for RIBF that occurred following the massive earthquake and tsunami that hit Japan in the spring of 2011. Another component of the research carried out with this grant involved developing the theoretical tools that are required

  10. Ionization Potentials for Isoelectronic Series.

    ERIC Educational Resources Information Center

    Agmon, Noam

    1988-01-01

    Presents a quantitative treatment of ionization potentials of isoelectronic atoms. By looking at the single-electron view of calculating the total energy of an atom, trends in the screening and effective quantum number parameters are examined. Approaches the question of determining electron affinities. (CW)

  11. Ionization Cooling for Muon Experiments

    SciTech Connect

    Alexahin, Y.; Neuffer, D.; Prebys, E.

    2014-09-18

    Possible application for muon experiments such as mu2e is discussed of the initial part of the ionization cooling channel originally developed for muon collider. It is shown that with the FNAL Booster as the proton driver the mu2e sensitivity can be increased by two orders of magnitude compared to the presently considered experiment.

  12. Electroencephalographic responses to ionizing radiation.

    PubMed

    GARCIA, J; BUCHWALD, N A; BACH-Y-RITA, G; FEDER, B H; KOELLING, R A

    1963-04-19

    Electroencephalographic recordings made from chronically implanted cortical electrodes indicate that ionizing radiation has an immediate effect upon brain wave patterns. X-rays delivered at the rate of 0.2 roentgen per second produce an arousal effect resembling that which occurs as a result of stimulation through peripheral receptor systems.

  13. Sterilization of skin allografts by ionizing radiation.

    PubMed

    Bourroul, Selma Cecília; Herson, Marisa Roma; Pino, Eddy; Matho, Monica Beatriz

    2002-11-01

    The skin has a fundamental role in the viability of human body. In the case of extensive wounds, skin allografts provide an alternative to cover temporarily the damaged areas. After donor screening and preservation in glycerol 85%, the skin can be stored in a Skin Bank. Glycerol at this concentration has a bacteriostatic effect after certain time of preservation. On the other hand, skin sterilization by ionizing radiation may reduce the quarentine period for transplantation in patients. The objective of this work was to evaluate allograft sterilization using two sources of ionizing radiation. Through the analysis of stress-strain, it was intended to verify possible effects of the radiation on the structure of preserved grafts. Three groups of skin samples were selected. The first group was maintained in the initial conditions, not irradiated. The second was exposed to cobalt-60, while the third one was irradiated using an Dynamitron Accelerator JOB188 electron beam. The irradiation dose was 25 kGy for both tests. Both irradiation sources, and the Instron Universal Machine used for biomechanical experiments, are installed at the Centro de Tecnologia das Radiações/Instituto de Pesquisas Energéticas e Nucleares (São Paulo, Brazil). According to the preliminary results, biomechanical characteristics of the samples irradiated seem to be maintained with regard to the non irradiated group.

  14. Capture and ionization detection of laser-cooled rubidium atoms with a charged suspended carbon nanotube

    NASA Astrophysics Data System (ADS)

    Ristroph, Trygve Gibbens

    The capture and ionization of neutral rubidium atoms with a positively charged suspended carbon nanotube is realized. The electric field surrounding the nanotube polarizes and pulls atoms into the highly singular attractive inverse square potential. Atoms are ionized by the nanotube, and Rb+ ions are ejected radially and subsequently detected individually. The entire process of capture, ionization, and ion-detection reveals a rich set of behavior, probing the dynamics of laser-cooled atoms as well as nanotube and ionization physics. When the device is used as an atom detector, the cold-atom ionization signal replicates time-dependent features in the instantaneous atom beam density on sub-millisecond time scales. This time resolution allows a time-of-flight measurement of atom velocity, corroborated with a laser absorption measurement. Position sensitivity on the 200 micron scale is demonstrated, as the detector is scanned to map out the atom beam transverse mode profile, a capability otherwise forbidden by the system's optical access. A measurement of the nanotube ionization cross-section as a function of atomic velocity and charging voltage shows the capture process is dominated by an inverse square potential energy. The cross-section reveals an inverse velocity scaling, consistent with the prediction. The analogous charging voltage measurement shows a linear scaling in voltage with measured and predicted slopes in agreement. Sending current through the nanotube changes the voltage offset of the cross-section versus voltage curve. This suggests that the ionization occurs in close proximity to the nanotube surface and is therefore sensitive to its electronic and mechanical properties. Theoretical foundations are developed to describe the capture and ionization physics involved in observing the quantization of atomic orbital angular momentum with the detector. For experimentally accessible parameters, the observation of the quantized conductance of neutral atoms is

  15. Clinical Application of Ambient Ionization Mass Spectrometry

    PubMed Central

    Li, Li-Hua; Hsieh, Hua-Yi; Hsu, Cheng-Chih

    2017-01-01

    Ambient ionization allows mass spectrometry analysis directly on the sample surface under atmospheric pressure with almost zero sample pretreatment. Since the development of desorption electrospray ionization (DESI) in 2004, many other ambient ionization techniques were developed. Due to their simplicity and low operation cost, rapid and on-site clinical mass spectrometry analysis becomes real. In this review, we will highlight some of the most widely used ambient ionization mass spectrometry approaches and their applications in clinical study. PMID:28337399

  16. Thermophysics Characterization of Multiply Ionized Air Plasma Absorption of Laser Radiation

    NASA Technical Reports Server (NTRS)

    Wang, Ten-See; Rhodes, Robert; Turner, Jim (Technical Monitor)

    2002-01-01

    The impact of multiple ionization of air plasma on the inverse Bremsstrahlung absorption of laser radiation is investigated for air breathing laser propulsion. Thermochemical properties of multiply ionized air plasma species are computed for temperatures up to 200,000 deg K, using hydrogenic approximation of the electronic partition function; And those for neutral air molecules are also updated for temperatures up to 50,000 deg K, using available literature data. Three formulas for absorption are calculated and a general formula is recommended for multiple ionization absorption calculation. The plasma composition required for absorption calculation is obtained by increasing the degree of ionization sequentially, up to quadruple ionization, with a series of thermal equilibrium computations. The calculated second ionization absorption coefficient agrees reasonably well with that of available data. The importance of multiple ionization modeling is demonstrated with the finding that area under the quadruple ionization curve of absorption is found to be twice that of single ionization. The effort of this work is beneficial to the computational plasma aerodynamics modeling of laser lightcraft performance.

  17. Multiphoton ionization studies of xenon clusters

    SciTech Connect

    Echt, O.; Cook, M.C.; Castleman, A.W.

    1987-04-03

    Non-resonant multiphoton ionization of xenon clusters has revealed the same magic numbers as found in the case of electron-impact ionization. Large dissociation rates are found for the trimer through pentamer ion, measured on a time scale of approx 10/sup -7/ s after ionization.

  18. 29 CFR 1926.53 - Ionizing radiation.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... 29 Labor 8 2014-07-01 2014-07-01 false Ionizing radiation. 1926.53 Section 1926.53 Labor... § 1926.53 Ionizing radiation. (a) In construction and related activities involving the use of sources of ionizing radiation, the pertinent provisions of the Nuclear Regulatory Commission's Standards for...

  19. 29 CFR 1926.53 - Ionizing radiation.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... 29 Labor 8 2012-07-01 2012-07-01 false Ionizing radiation. 1926.53 Section 1926.53 Labor... § 1926.53 Ionizing radiation. (a) In construction and related activities involving the use of sources of ionizing radiation, the pertinent provisions of the Nuclear Regulatory Commission's Standards for...

  20. 29 CFR 1926.53 - Ionizing radiation.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... 29 Labor 8 2011-07-01 2011-07-01 false Ionizing radiation. 1926.53 Section 1926.53 Labor... § 1926.53 Ionizing radiation. (a) In construction and related activities involving the use of sources of ionizing radiation, the pertinent provisions of the Nuclear Regulatory Commission's Standards for...

  1. 29 CFR 1926.53 - Ionizing radiation.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 29 Labor 8 2010-07-01 2010-07-01 false Ionizing radiation. 1926.53 Section 1926.53 Labor... § 1926.53 Ionizing radiation. (a) In construction and related activities involving the use of sources of ionizing radiation, the pertinent provisions of the Nuclear Regulatory Commission's Standards for...

  2. 29 CFR 1926.53 - Ionizing radiation.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... 29 Labor 8 2013-07-01 2013-07-01 false Ionizing radiation. 1926.53 Section 1926.53 Labor... § 1926.53 Ionizing radiation. (a) In construction and related activities involving the use of sources of ionizing radiation, the pertinent provisions of the Nuclear Regulatory Commission's Standards for...

  3. Advanced Quantification of Plutonium Ionization Potential to Support Nuclear Forensic Evaluations by Resonance Ionization Mass Spectrometry

    DTIC Science & Technology

    2015-06-01

    QUANTIFICATION OF PLUTONIUM IONIZATION POTENTIAL TO SUPPORT NUCLEAR FORENSIC EVALUATIONS BY RESONANCE IONIZATION MASS SPECTROMETRY by Craig T...PLUTONIUM IONIZATION POTENTIAL TO SUPPORT NUCLEAR FORENSIC EVALUATIONS BY RESONANCE IONIZATION MASS SPECTROMETRY 5. FUNDING NUMBERS 6. AUTHOR(S...mass spectrometry (RIMS) to problems related to nuclear forensics and, in particular, to the analysis and quantification of the debris from nuclear

  4. Electron-Impact Ionization and Dissociative Ionization of Biomolecules

    NASA Technical Reports Server (NTRS)

    Huo, Winifred M.; Chaban, Galina M.; Dateo, Christopher E.

    2006-01-01

    It is well recognized that secondary electrons play an important role in radiation damage to humans. Particularly important is the damage of DNA by electrons, potentially leading to mutagenesis. Molecular-level study of electron interaction with DNA provides information on the damage pathways and dominant mechanisms. Our study of electron-impact ionization of DNA fragments uses the improved binary-encounter dipole model and covers DNA bases, sugar phosphate backbone, and nucleotides. An additivity principle is observed. For example, the sum of the ionization cross sections of the separate deoxyribose and phosphate fragments is in close agreement with the C3(sup prime)- and C5 (sup prime)-deoxyribose-phospate cross sections, differing by less than 5%. Investigation of tandem double lesion initiated by electron-impact dissociative ionization of guanine, followed by proton reaction with the cytosine in the Watson-Crick pair, is currently being studied to see if tandem double lesion can be initiated by electron impact. Up to now only OH-induced tandem double lesion has been studied.

  5. Electron-Impact Ionization and Dissociative Ionization of Biomolecules

    NASA Technical Reports Server (NTRS)

    Huo, Winifred M.; Chaban, Galina M.; Dateo, Christopher E.

    2006-01-01

    It is well recognized that secondary electrons play an important role in radiation damage to humans. Particularly important is the damage of DNA by electrons, potentially leading to mutagenesis. Molecular-level study of electron interaction with DNA provides information on the damage pathways and dominant mechanisms. Our study of electron-impact ionization of DNA fragments uses the improved binary-encounter dipole model and covers DNA bases, sugar phosphate backbone, and nucleotides. An additivity principle is observed. For example, the sum of the ionization cross sections of the separate deoxyribose and phosphate fragments is in close agreement with the C3(sup prime)- and C5 (sup prime)-deoxyribose-phospate cross sections, differing by less than 5%. Investigation of tandem double lesion initiated by electron-impact dissociative ionization of guanine, followed by proton reaction with the cytosine in the Watson-Crick pair, is currently being studied to see if tandem double lesion can be initiated by electron impact. Up to now only OH-induced tandem double lesion has been studied.

  6. Position sensitive disc for charged particle detection

    NASA Astrophysics Data System (ADS)

    Bellini, V.; Palazzolo, F.; Scirè, A.; Sperduto, M. L.; Albergo, S.; Poli, G.; Potenza, R.; Randieri, C.; Russo, V.; Sutera, M. C.; Capogni, M.; Schaerf, C.; D'Angelo, A.; Moricciani, D.; Kuznetsov, A. V.; Girolami, B.; Ghio, F.

    2001-04-01

    A plastic scintillating disc (NE102, 3 cm thick, 1 m diameter) has been designed for detecting charged pions in nuclear reactions at intermediate energy. A hole of 20 cm diameter was made in the middle of the disc in order to allow for the beam passage through the detector. The originality of the detector consists of the simultaneous use of four very compact central Photo Multiplier Tubes (PMT) and eight peripheral PMTs in order to retrieve the hitting point of a charged particle onto the disc surface with a space resolution of ±3 cm. The original method has been developed by using polar coordinates and only the Time-Of-Flight information (TOF) from three or four nearest PMTs, including at least one central PMT.

  7. Position sensitive counter development at the linac

    SciTech Connect

    Becker, J.A.

    1981-05-20

    In a novel application of the multiwire proportional counter we have imaged a collimated neutron beam. Although preliminary, the results are of sufficient import to be described here because of the potential wide application of the multiwire proportional counter to Laboratory problems. The counter was operated with a counting gas pressure of 20 Torr; the counting gas was pure C/sub 4/H/sub 10/. The radiator was a /sup 235/U foil. Under these conditions, the counter is (1) relatively insensitive to charged particles (other than fission fragments), (2) insensitive to ..gamma..-radiation, and (3) has an efficiency for the detection of fission fragments independent of incident neutron energy over a wide range of neutron energies.

  8. Neutron position-sensitive scintillation detector

    DOEpatents

    Strauss, Michael G.; Brenner, Raul

    1984-01-01

    A device is provided for mapping one- and two-dimensional distributions of neutron-positions in a scintillation detector. The device consists of a lithium glass scintillator coupled by an air gap and a light coupler to an array of photomultipliers. The air gap concentrates light flashes from the scintillator, whereas the light coupler disperses this concentrated light to a predetermined fraction of the photomultiplier tube array.

  9. Ionizing radiation and cancer prevention.

    PubMed Central

    Hoel, D G

    1995-01-01

    Ionizing radiation long has been recognized as a cause of cancer. Among environmental cancer risks, radiation is unique in the variety of organs and tissues that it can affect. Numerous epidemiological studies with good dosimetry provide the basis for cancer risk estimation, including quantitative information derived from observed dose-response relationships. The amount of cancer attributable to ionizing radiation is difficult to estimate, but numbers such as 1 to 3% have been suggested. Some radiation-induced cancers attributable to naturally occurring exposures, such as cosmic and terrestrial radiation, are not preventable. The major natural radiation exposure, radon, can often be reduced, especially in the home, but not entirely eliminated. Medical use of radiation constitutes the other main category of exposure; because of the importance of its benefits to one's health, the appropriate prevention strategy is to simply work to minimize exposures. PMID:8741791

  10. L -shell ionization by antiprotons

    SciTech Connect

    Sarkadi, L. , H-4001 Debrecen, Pf. 51, Hungary ); Mukoyama, T. )

    1990-10-01

    Semiclassical coupled-state model calculations have been performed for {ital L}-shell ionization of gold induced by protons and antiprotons in the energy range 0.15--3 MeV. The results of the calculations have been compared with the predictions of a simple approach suggested by Brandt and Basbas for description of antiparticle excitation of atomic inner shells. Apart from the range of very low collision velocities, a reasonable agreement has been found between the two models. In addition to the binding and Coulomb-distortion effects discussed by Brandt and Basbas (Phys. Rev. A 27, 578 (1983); 28, 3142(E) (1983)), for the {ital L} shell a further effect due to dynamical couplings between the {ital L}-substate ionization amplitudes also contributes to the particle-antiparticle differences. While the latter processes have only a negligible effect on the energy dependence of the cross sections, their inclusion has been shown to be unavoidable when ratios of the subshell ionization cross sections are analyzed for the two kinds of excitation.

  11. Low-density ionization behavior

    SciTech Connect

    Baker, G.A. Jr.

    1995-04-01

    As part of a continuing study of the physics of matter under extreme conditions, I give some results on matter at extremely low density. In particular I compare a quantum mechanical calculation of the pressure for atomic hydrogen with the corresponding pressure given by Thomas-Fermi theory. (This calculation differs from the ``confined atom`` approximation in a physically significant way.) Since Thomas-Fermi theory in some sense, represents the case of infinite nuclear charge, these cases should represent extremes. Comparison is also made with Saha theory, which considers ionization from a chemical point of view, but is weak on excited-state effects. In this theory, the pressure undergoes rapid variation as electron ionization levels are passed. This effect is in contrast to the smooth behavior of the Thomas-Fermi fixed temperature, complete ionization occurs in the low density limit, I study the case where the temperature goes appropriately to zero with the density. Although considerable modification is required, Saha theory is closer to the actual results for this case than is Thomas-Fermi theory.

  12. Theory of dissociative tunneling ionization

    NASA Astrophysics Data System (ADS)

    Svensmark, Jens; Tolstikhin, Oleg I.; Madsen, Lars Bojer

    2016-05-01

    We present a theoretical study of the dissociative tunneling ionization process. Analytic expressions for the nuclear kinetic energy distribution of the ionization rates are derived. A particularly simple expression for the spectrum is found by using the Born-Oppenheimer (BO) approximation in conjunction with the reflection principle. These spectra are compared to exact non-BO ab initio spectra obtained through model calculations with a quantum mechanical treatment of both the electronic and nuclear degrees of freedom. In the regime where the BO approximation is applicable, imaging of the BO nuclear wave function is demonstrated to be possible through reverse use of the reflection principle, when accounting appropriately for the electronic ionization rate. A qualitative difference between the exact and BO wave functions in the asymptotic region of large electronic distances is shown. Additionally, the behavior of the wave function across the turning line is seen to be reminiscent of light refraction. For weak fields, where the BO approximation does not apply, the weak-field asymptotic theory describes the spectrum accurately.

  13. Ionization-based detectors for gas chromatography.

    PubMed

    Poole, Colin F

    2015-11-20

    The gas phase ionization detectors are the most widely used detectors for gas chromatography. The column and makeup gases commonly used in gas chromatography are near perfect insulators. This facilitates the detection of a minute number of charge carriers facilitating the use of ionization mechanisms of low efficiency while providing high sensitivity. The main ionization mechanism discussed in this report are combustion in a hydrogen diffusion flame (flame ionization detector), surface ionization in a plasma (thermionic ionization detector), photon ionization (photoionization detector and pulsed discharge helium ionization detector), attachment of thermal electrons (electron-capture detector), and ionization by collision with metastable helium species (helium ionization detector). The design, response characteristics, response mechanism, and suitability for fast gas chromatography are the main features summarized in this report. Mass spectrometric detection and atomic emission detection, which could be considered as ionization detectors of a more sophisticated and complex design, are not discussed in this report. Copyright © 2015 Elsevier B.V. All rights reserved.

  14. Polarization phenomena in multiphoton ionization of atoms.

    NASA Technical Reports Server (NTRS)

    Jacobs, V. L.

    1973-01-01

    The theory of multiphoton ionization for an atomic system of arbitrary complexity is developed using a density matrix formalism. An expression is obtained which determines the differential N-photon ionization cross section as a function of the polarization states of the target atom and the incident radiation. The parameters which characterize the photo-electron angular distribution are related to the general reduced matrix elements for the N-photon transition. Two-photon ionization of unpolarized atoms is treated as an illustration of the use of the theory. The dependence of the multiphoton ionization cross section on the polarization state of the incident radiation, which has been observed in two- and three-photon ionization of Cs, is accounted for by the theory. Finally, the photoelectron spin polarization produced by the multiphoton ionization of unpolarized atoms, like the analogous polarization resulting from single-photon ionization, is found to depend on the circular polarization of the incident radiation.

  15. Polarization phenomena in multiphoton ionization of atoms

    NASA Technical Reports Server (NTRS)

    Jacobs, V. L.

    1973-01-01

    The theory of multiphoton ionization for an atomic system of arbitrary complexity is developed using a density matrix formalism. An expression is obtained which determines the differential N-photon ionization cross section as a function of the polarization states of the target atom and the incident radiation. The parameters which characterize the photoelectron angular distribution are related to the general reduced matrix elements for the N-photon transition. Two-photon ionization of unpolarized atoms is treated as an illustration of the use of the theory. The dependence of the multiphoton ionization cross section on the polarization state of the incident radiation, which has been observed in two- and three-photon ionization of Cs, is accounted for by the theory. Finally, the photoelectron spin polarization produced by the multiphoton ionization of unpolarized atoms, like the analogous polarization resulting from single-photon ionization, is found to depend on the circular polarization of the incident radiation.

  16. Turbulence and the ionization of interstellar gas

    NASA Astrophysics Data System (ADS)

    Hill, Alex S.

    2015-08-01

    Turbulence is widely observed in the ionized gas in the interstellar media of star-forming galaxies. Observations in the Milky Way indicate emission from that the warm ionized medium -- ionized gas far from massive stars, the most likely source of the ionization -- has a lognormal intensity distribution. This and other measurements indicate that the gas is well-described as a transonic turbulent fluid. Such a fluid can be produced by feedback from supernovae in the Galaxy. Understanding of this turbulence has also led to a natural explanation for a long-standing puzzle: how do ionizing photons travel through the largely-neutral interstellar medium and produce the ionization? In the turbulent gas, low-density pathways allow ionizing photons to propagate for kiloparsecs, with implications for radiative energy transport in star-forming galaxies.

  17. Ionizing Radiation and Its Risks

    PubMed Central

    Goldman, Marvin

    1982-01-01

    Penetrating ionizing radiation fairly uniformly puts all exposed molecules and cells at approximately equal risk for deleterious consequences. Thus, the original deposition of radiation energy (that is, the dose) is unaltered by metabolic characteristics of cells and tissue, unlike the situation for chemical agents. Intensely ionizing radiations, such as neutrons and alpha particles, are up to ten times more damaging than sparsely ionizing sources such as x-rays or gamma rays for equivalent doses. Furthermore, repair in cells and tissues can ameliorate the consequences of radiation doses delivered at lower rates by up to a factor of ten compared with comparable doses acutely delivered, especially for somatic (carcinogenic) and genetic effects from x- and gamma-irradiation exposure. Studies on irradiated laboratory animals or on people following occupational, medical or accidental exposures point to an average lifetime fatal cancer risk of about 1 × 10-4 per rem of dose (100 per 106 person-rem). Leukemia and lung, breast and thyroid cancer seem more likely than other types of cancer to be produced by radiation. Radiation exposures from natural sources (cosmic rays and terrestrial radioactivity) of about 0.1 rem per year yield a lifetime cancer risk about 0.1 percent of the normally occurring 20 percent risk of cancer death. An increase of about 1 percent per rem in fatal cancer risk, or 200 rem to double the “background” risk rate, is compared with an estimate of about 100 rem to double the genetic risk. Newer data suggest that the risks for low-level radiation are lower than risks estimated from data from high exposures and that the present 5 rem per year limit for workers is adequate. PMID:6761969

  18. The Tevatron Ionization Profile Monitors

    SciTech Connect

    Jansson, A.; Fitzpatrick, T.; Bowie, K.; Kwarciany, R.; Lundberg, C.; Slimmer, D.; Valerio, L.; Zagel, J.; /Fermilab

    2006-05-01

    In designing an ionization profile monitor system for the Tevatron some novel approaches were taken, in particular for the readout electronics. This was motivated by the desire to resolve the individual bunches in both beams simultaneously. For this purpose, custom made electronics originally developed for Particle Physics experiments was used to provide a fast charge integration with very low noise. The various parts of the read-out electronics have been borrowed or adapted from the KTev, CMS, MINOS and BTev experiments. The detector itself also had to be modified to provide clean signals with sufficient bandwidth. The system design will be described along with the initial results.

  19. Space Flight Ionizing Radiation Environments

    NASA Technical Reports Server (NTRS)

    Koontz, Steve

    2017-01-01

    The space-flight ionizing radiation (IR) environment is dominated by very high-kinetic energy-charged particles with relatively smaller contributions from X-rays and gamma rays. The Earth's surface IR environment is not dominated by the natural radioisotope decay processes. Dr. Steven Koontz's lecture will provide a solid foundation in the basic engineering physics of space radiation environments, beginning with the space radiation environment on the International Space Station and moving outward through the Van Allen belts to cislunar space. The benefits and limitations of radiation shielding materials will also be summarized.

  20. XUV ionization of aligned molecules

    SciTech Connect

    Kelkensberg, F.; Siu, W.; Gademann, G.; Rouzee, A.; Vrakking, M. J. J.; Johnsson, P.; Lucchini, M.; Lucchese, R. R.

    2011-11-15

    New extreme-ultraviolet (XUV) light sources such as high-order-harmonic generation (HHG) and free-electron lasers (FELs), combined with laser-induced alignment techniques, enable novel methods for making molecular movies based on measuring molecular frame photoelectron angular distributions. Experiments are presented where CO{sub 2} molecules were impulsively aligned using a near-infrared laser and ionized using femtosecond XUV pulses obtained by HHG. Measured electron angular distributions reveal contributions from four orbitals and the onset of the influence of the molecular structure.

  1. Advanced Thin Ionization Calorimeter (ATIC)

    NASA Technical Reports Server (NTRS)

    Wefel, John P.

    1998-01-01

    This is the final report for NASA grant NAGW-4577, "Advanced Thin Ionization Calorimeter (ATIC)". This grant covered a joint project between LSU and the University of Maryland for a Concept Study of a new type of fully active calorimeter to be used to measure the energy spectra of very high energy cosmic rays, particularly Hydrogen and Helium, to beyond 1014 eV. This very high energy region has been studied with emulsion chamber techniques, but never investigated with electronic calorimeters. Technology had advanced to the point that a fully active calorimeter based upon Bismuth Germanate (BGO) scintillating crystals appeared feasible for balloon flight (and eventually space) experiments.

  2. Superponderomotive regime of tunneling ionization

    NASA Astrophysics Data System (ADS)

    Gordon, D. F.; Palastro, J. P.; Hafizi, B.

    2017-03-01

    Ultrarelativistic photoelectron spectra exhibit unexpected characteristics in a paraxial laser focus. The photoelectron energy scales superponderomotively, and the usual parabolic momentum distribution is distorted into a variety of intricate patterns, depending on the location of the ion. These patterns include discrete contours, which in some cases can be easily identified with a particular subcycle burst of ionization current. An analytical formula for the maximum photoelectron energy in a paraxial radiation field is given, and high-resolution momentum distributions with narrowly peaked features are presented. These narrowly peaked features suggest application to electron injection into plasma-based accelerators.

  3. Ionization of cationic micelles: effect of the detergent structure

    SciTech Connect

    Zana, R.

    1980-12-01

    Measurements show that the micelle ionization degree decreases upon increasing chain length in the alkyltrimethylammonium bromides series, increases with the size of the ionic head group in the tetradecyltrialkylammonium bromide series, and with the length of the variable alkyl chain in the dodecyldimethylalkylammonium bromide series. These variations have been explained in terms of changes of surface area per head group calculated on the basis of a model which assumes spherical micelles. 34 references.

  4. Generation of monoenergetic ion beams via ionization dynamics (Conference Presentation)

    NASA Astrophysics Data System (ADS)

    Lin, Chen; Kim, I. Jong; Yu, Jinqing; Choi, Il Woo; Ma, Wenjun; Yan, Xueqing; Nam, Chang Hee

    2017-05-01

    The research on ion acceleration driven by high intensity laser pulse has attracted significant interests in recent decades due to the developments of laser technology. The intensive study of energetic ion bunches is particularly stimulated by wide applications in nuclear fusion, medical treatment, warm dense matter production and high energy density physics. However, to implement such compact accelerators, challenges are still existing in terms of beam quality and stability, especially in applications that require higher energy and narrow bandwidth spectra ion beams. We report on the acceleration of quasi-mono-energetic ion beams via ionization dynamics in the interaction of an intense laser pulse with a solid target. Using ionization dynamics model in 2D particle-in-cell (PIC) simulations, we found that high charge state contamination ions can only be ionized in the central spot area where the intensity of sheath field surpasses their ionization threshold. These ions automatically form a microstructure target with a width of few micron scale, which is conducive to generate mono-energetic beams. In the experiment of ultraintense (< 10^21 W/cm^2) laser pulses irradiating ultrathin targets each attracted with a contamination layer of nm-thickness, high quality < 100 MeV mono-energetic ion bunches are generated. The peak energy of the self-generated micro-structured target ions with respect to different contamination layer thickness is also examined This is relatively newfound respect, which is confirmed by the consistence between experiment data and the simulation results.

  5. Field Ionization detection of supersonic helium atom beams

    NASA Astrophysics Data System (ADS)

    Doak, R. B.

    2003-10-01

    Field ionization detectors (FID) may offer near-unity detection efficiency and nanoscale spatial resolution. To date, FID detection of molecular beams has been limited to effusive beams of broad Maxwellian velocity distributions. We report FID measurements on monoenergetic helium beams, including intensity measurements and time-of-flight measurements. The FID tips were carefully prepared and characterized in a field ionization microscope prior to use. With the supersonic helium beam we find a much smaller effective detection area ( 50 sq. nm) than was reported in the effusive helium beam experiments ( 200,000 sq. nm). This suggests that the FID ionization yield depends strongly on energy loss by the impinging atom during its initial collision with the FID surface: Our thermal energy, monoenergetic helium beam atoms likely lose little or no energy upon scattering from the clean tungsten FID surface, allowing the scattered atoms to escape the FID polarization field and therby reducing the ionization yield. To improve signal levels, inelastic scattering might be enhanced by use of lower beam velocities (present in the tails of a Maxwellian) or by adsorbing an overlayer on the FID tip (present at cryogenic tip temperatures). These factors likely explain the higher detection yields measured in the effusive beam experiments.

  6. HF Accelerated Electron Fluxes, Spectra, and Ionization

    NASA Astrophysics Data System (ADS)

    Carlson, Herbert C.; Jensen, Joseph B.

    2015-10-01

    Wave particle interactions, an essential aspect of laboratory, terrestrial, and astrophysical plasmas, have been studied for decades by transmitting high power HF radio waves into Earth's weakly ionized space plasma, to use it as a laboratory without walls. Application to HF electron acceleration remains an active area of research (Gurevich in Usp Fizicheskikh Nauk 177(11):1145-1177, 2007) today. HF electron acceleration studies began when plasma line observations proved (Carlson et al. in J Atmos Terr Phys 44:1089-1100, 1982) that high power HF radio wave-excited processes accelerated electrons not to ~eV, but instead to -100 times thermal energy (10 s of eV), as a consequence of inelastic collision effects on electron transport. Gurevich et al (J Atmos Terr Phys 47:1057-1070, 1985) quantified the theory of this transport effect. Merging experiment with theory in plasma physics and aeronomy, enabled prediction (Carlson in Adv Space Res 13:1015-1024, 1993) of creating artificial ionospheres once ~GW HF effective radiated power could be achieved. Eventual confirmation of this prediction (Pedersen et al. in Geophys Res Lett 36:L18107, 2009; Pedersen et al. in Geophys Res Lett 37:L02106, 2010; Blagoveshchenskaya et al. in Ann Geophys 27:131-145, 2009) sparked renewed interest in optical inversion to estimate electron spectra in terrestrial (Hysell et al. in J Geophys Res Space Phys 119:2038-2045, 2014) and planetary (Simon et al. in Ann Geophys 29:187-195, 2011) atmospheres. Here we present our unpublished optical data, which combined with our modeling, lead to conclusions that should meaningfully improve future estimates of the spectrum of HF accelerated electron fluxes. Photometric imaging data can significantly improve detection of emissions near ionization threshold, and confirm depth of penetration of accelerated electrons many km below the excitation altitude. Comparing observed to modeled emission altitude shows future experiments need electron density profiles

  7. Atmospheric sampling glow discharge ionization source

    DOEpatents

    McLuckey, S.A.; Glish, G.L.

    1989-07-18

    An atmospheric sampling glow discharge ionization source that can be used in combination with an analytical instrument which operates at high vacuum, such as a mass spectrometer. The atmospheric sampling glow discharge ionization source comprises a chamber with at least one pair of electrodes disposed therein, an inlet for a gaseous sample to be analyzed and an outlet communicating with an analyzer which operates at subatmospheric pressure. The ionization chamber is maintained at a pressure below atmospheric pressure, and a voltage difference is applied across the electrodes to induce a glow discharge between the electrodes, so that molecules passing through the inlet are ionized by the glow discharge and directed into the analyzer. The ionization source accepts the sample under atmospheric pressure conditions and processes it directly into the high vacuum instrument, bridging the pressure gap and drawing off unwanted atmospheric gases. The invention also includes a method for analyzing a gaseous sample using the glow discharge ionization source described above. 3 figs.

  8. Fluid hydrogen at high density - Pressure ionization

    NASA Technical Reports Server (NTRS)

    Saumon, Didier; Chabrier, Gilles

    1992-01-01

    The Helmholtz-free-energy model for nonideal mixtures of hydrogen atoms and molecules by Saumon and Chabrier (1991) is extended to describe dissociation and ionization in similar mixtures in chemical equilibrium. A free-energy model is given that describes partial ionization in the pressure and temperature ionization region. The plasma-phase transition predicted by the model is described for hydrogen mixtures including such components as H2, H, H(+), and e(-). The plasma-phase transition has a critical point at Tc = 15,300 K and Pc = 0.614 Mbar, and thermodynamic instability is noted in the pressure-ionization regime. The pressure dissociation and ionization of fluid hydrogen are described well with the model yielding information on the nature of the plasma-phase transition. The model is shown to be valuable for studying dissociation and ionization in astrophysical objects and in high-pressure studies where pressure and temperature effects are significant.

  9. Electron ionization of H2O

    NASA Astrophysics Data System (ADS)

    King, Simon J.; Price, Stephen D.

    2008-11-01

    Relative partial ionization cross-sections and precursor-specific relative partial ionization cross-sections for fragment ions formed by electron ionization of H2O have been measured using time-of-flight mass spectrometry coupled with a 2D ion coincidence technique. We report data for the formation of H+, H2+, O2+, O+ and OH+ relative to the formation of H2O+, as a function of ionizing electron energy from 30 to 200 eV. This data includes, for the first time, measurements on the formation all positive ion pairs and ion triples by dissociative multiple electron ionization of H2O. Through determinations of the kinetic energy release involved in ion pair formation we provide further evidence that indirect processes contribute significantly to the yield of H+ + OH+ ion pairs below the vertical double ionization threshold.

  10. Atmospheric sampling glow discharge ionization source

    DOEpatents

    McLuckey, Scott A.; Glish, Gary L.

    1989-01-01

    An atmospheric sampling glow discharge ionization source that can be used in combination with an analytical instrument which operates at high vacuum, such as a mass spectrometer. The atmospheric sampling glow discharge ionization source comprises a chamber with at least one pair of electrodes disposed therein, an inlet for a gaseous sample to be analyzed and an outlet communicating with an analyzer which operates at subatmospheric pressure. The ionization chamber is maintained at a pressure below atmospheric pressure, and a voltage difference is applied across the electrodes to induce a glow discharge between the electrodes, so that molecules passing through the inlet are ionized by the glow discharge and directed into the analyzer. The ionization source accepts the sample under atmospheric pressure conditions and processes it directly into the high vacuum instrument, bridging the pressure gap and drawing off unwanted atmospheric gases. The invention also includes a method for analyzing a gaseous sample using the glow discharge ionization source described above.

  11. Multiphoton Ionization Mass and Photoelectron Spectroscopy.

    DTIC Science & Technology

    1984-07-01

    narro , band. tunable. frequency doubled dye laser Their relative importance depend% on the sample being studied ha- led to an cnormou, improcment in...block number) Mult iphoton Ionization Photoelectron Spectroscopy Laser Induced Ionization Ultraviolet Laser Radiation ft ArITAcr (camthIe i rvee ehl N...molecular ions generated by laser ionization have been monitored. Using a time of flight photoelectron spectrometer, the kinetic energy distribution of the

  12. Atomic inner-shell ionization

    NASA Astrophysics Data System (ADS)

    Das, J. N.; Chakraborty, S.

    1985-07-01

    Cross sections for the K-shell ionization of medium-heavy atoms by relativistic electrons have been calculated in a relativistic framework in the Coulomb gauge to order α0 (=e2/ħc) in the interaction Hamiltonian. Here exchange is neglected. The incident- and scattered-electron wave functions are described by Dirac plane waves. Only the bound- and ejected-electron wave functions are described nonrelativistically for a screened Coulomb potential, used earlier by the present authors. Thus the screening effect is taken into account in this calculation in a satisfactory manner. The calculation is a repetition of what has been published recently by the present authors with one important exception: Here, the ejected-electron continuum state wave function that is used is determined variationally for the above screened Coulomb potential. Thereby some perturbation approximation of ad hoc nature could be avoided. As a consequence, considerable improvement is noticed in the total cross-section results. Comparison with experimental results for 29Cu, 47Ag, and 79Au shows a good agreement. The calculation may easily be extended to ionization from other shells.

  13. Ionizing radiation and orthopaedic prostheses

    NASA Astrophysics Data System (ADS)

    Rimnac, Clare M.; Kurtz, Steven M.

    2005-07-01

    Ultra high molecular weight polyethylene (UHMWPE) materials have been used successfully as one half of the bearing couple (against metallic alloys or ceramics) in total hip and total knee joint replacements for four decades. This review describes the impact of ionizing radiation (used for sterilization and for microstructural modification via crosslinking) on the performance of UHMWPE total joint replacement components. Gamma radiation sterilization in air leads to oxidative degradation of UHMWPE joint components that occurs during shelf-aging and also during in vivo use. Efforts to mitigate oxidative degradation of UHMWPE joint components include gamma radiation sterilization in inert barrier-packaging and processing treatments to reduce free radicals. Ionizing radiation (both gamma and electron-beam) has recently been used to form highly crosslinked UHMWPEs that have better adhesive and abrasive wear resistance than non-crosslinked UHMWPE, thereby potentially improving the long-term performance of total joint replacements. Along with increased wear resistance, however, there are deleterious changes to ductility and fracture resistance of UHMWPE, and an increased risk of fracture of these components remains a clinical concern.

  14. NMR Metabolomics in Ionizing Radiation

    SciTech Connect

    Hu, Jian Z.; Xiao, Xiongjie; Hu, Mary Y.

    2016-09-08

    Ionizing radiation is an invisible threat that cannot be seen, touched or smelled and exist either as particles or waves. Particle radiation can take the form of alpha, beta or neutrons, as well as high energy space particle radiation such as high energy iron, carbon and proton radiation, etc. (1) Non-particle radiation includes gamma- and x-rays. Publically, there is a growing concern about the adverse health effects due to ionizing radiation mainly because of the following facts. (a) The X-ray diagnostic images are taken routinely on patients. Even though the overall dosage from a single X-ray image such as a chest X-ray scan or a CT scan, also called X-ray computed tomography (X-ray CT), is low, repeated usage can cause serious health consequences, in particular with the possibility of developing cancer (2, 3). (b) Human space exploration has gone beyond moon and is planning to send human to the orbit of Mars by the mid-2030s. And a landing on Mars will follow.

  15. Sequential binary collision ionization mechanisms

    NASA Astrophysics Data System (ADS)

    van Boeyen, R. W.; Watanabe, N.; Doering, J. P.; Moore, J. H.; Coplan, M. A.; Cooper, J. W.

    2004-03-01

    Fully differential cross sections for the electron-impact ionization of the magnesium 3s orbital have been measured in a high-momentum-transfer regime wherein the ionization mechanisms can be accurately described by simple binary collision models. Measurements where performed at incident-electron energies from 400 to 3000 eV, ejected-electron energies of 62 eV, scattering angle of 20 °, and momentum transfers of 2 to 5 a.u. In the out-of-plane geometry of the experiment the cross section is observed far off the Bethe ridge. Both first- and second-order processes can be clearly distinguished as previously observed by Murray et al [Ref. 1] and Schulz et al [Ref. 2]. Owing to the relatively large momentum of the ejected electron, the second order processes can be modeled as sequential binary collisions involving a binary elastic collision between the incident electron and ionic core and a binary knock-out collision between the incident electron and target electron. At low incident-electron energies the cross section for both first and second order processes are comparable, while at high incident energies second-order processes dominate. *Supported by NSF under grant PHY-99-87870. [1] A. J. Murray, M. B. J. Woolf, and F. H. Read J. Phys. B 25, 3021 (1992). [2] M. Schulz, R. Moshammer, D. Fischer, H. Kollmus, D. H. Madison. S. Jones and J. Ullrich, Nature 422, 48 (2003).

  16. Ionization probes of molecular structure and chemistry

    SciTech Connect

    Johnson, P.M.

    1993-12-01

    Various photoionization processes provide very sensitive probes for the detection and understanding of the spectra of molecules relevant to combustion processes. The detection of ionization can be selective by using resonant multiphoton ionization or by exploiting the fact that different molecules have different sets of ionization potentials. Therefore, the structure and dynamics of individual molecules can be studied even in a mixed sample. The authors are continuing to develop methods for the selective spectroscopic detection of molecules by ionization, and to use these methods for the study of some molecules of combustion interest.

  17. Initial results of positron ionization mass spectrometry

    NASA Technical Reports Server (NTRS)

    Donohue, D. L.; Hulett, L. D., Jr.; Mcluckey, S. A.; Glish, G. L.; Eckenrode, B. A.

    1990-01-01

    The use of monoenergetic positrons for the ionization of organic molecules in the gas phase is described. The ionic products are analyzed with a time-of-flight mass spectrometer and detected to produce a mass spectrum. The ionization mechanisms which can be studied in this way include positron impact at energies above the ionization limit of the target molecules, positronium formation in the Ore gap energy range, and positron attachment at energies less than 1eV. The technique of positron ionization mass spectrometry (PIMS) may have analytical utility in that chemical selectivity is observed for one or more of these processes.

  18. New design of high performance ionizing bar

    NASA Astrophysics Data System (ADS)

    Wang, Ronggang; Sun, Yurong

    2013-03-01

    This paper introduces a new design of DC-pulse ionizing bar to solve the problem of imbalance offset voltage for the AC ionizing bar, which is easily affected by the environment, as well as indicate the final tests. The new design mainly includes five parts: power supply circuit, main control unit, logic circuit, high frequency transformer unit, and feedback unit. The ionizing bar can automatically adjust the discharge voltage, pulse frequency and pulse width to balance the positive and negative ions. The final test results indicate that the DC ionizing bar owns good effect in electrostatic elimination.

  19. Tunneling ionization time-resolved by backpropagation

    NASA Astrophysics Data System (ADS)

    Ni, Hongcheng; Saalmann, Ulf; Rost, Jan M.; Max-Planck-Institut für Physik komplexer Systeme Team

    2016-05-01

    We determine the ionization time in tunneling ionization by an elliptically polarized light pulse relative to its maximum. This is achieved by a full quantum propagation of the electron wave function forward in time, followed by a classical backpropagation to identify tunneling parameters, in particular the fraction of electrons that has tunneled out. We find, that the ionization time is close to zero for single active electrons in helium and in hydrogen if the fraction of tunneled electrons is large. We expect our analysis to be essential to quantify ionization times for correlated electron motion. This work was supported by Alexander von Humboldt Foundation.

  20. Influence of renormalization shielding on the electron-impact ionization process in dense partially ionized plasmas

    SciTech Connect

    Song, Mi-Young; Yoon, Jung-Sik; Jung, Young-Dae

    2015-04-15

    The renormalization shielding effects on the electron-impact ionization of hydrogen atom are investigated in dense partially ionized plasmas. The effective projectile-target interaction Hamiltonian and the semiclassical trajectory method are employed to obtain the transition amplitude as well as the ionization probability as functions of the impact parameter, the collision energy, and the renormalization parameter. It is found that the renormalization shielding effect suppresses the transition amplitude for the electron-impact ionization process in dense partially ionized plasmas. It is also found that the renormalization effect suppresses the differential ionization cross section in the peak impact parameter region. In addition, it is found that the influence of renormalization shielding on the ionization cross section decreases with an increase of the relative collision energy. The variations of the renormalization shielding effects on the electron-impact ionization cross section are also discussed.

  1. Specific heparin preparations interfere with the simultaneous measurement of ionized magnesium and ionized calcium.

    PubMed

    Lyon, M E; Bremner, D; Laha, T; Malik, S; Henderson, P J; Kenny, M A

    1995-02-01

    To determine whether heparin anticoagulants used for analysis of whole blood ionized calcium would influence the measurement of ionized magnesium. The effects of zinc heparin, lithium heparin, and electrolyte-balanced heparin on the simultaneous measurement of ionized magnesium and ionized calcium in serum were determined using ion selective electrodes. Time-dependent biases in ionized magnesium and calcium concentrations were apparent with zinc heparin but not with lithium or electrolyte-balanced heparin. Ionized magnesium and calcium concentrations were more significantly influenced by volume-dependent changes in zinc heparin potency than with lithium or electrolyte-balanced heparin. Zinc heparin produces a significant positive bias in the simultaneous determination of ionized magnesium and ionized calcium concentrations.

  2. Ionizing radiation effects on silicon test structures

    SciTech Connect

    Kraner, H.W.; Beuttenmuller, R.; Chen, W.; Kierstead, J.A.; Li, Z.; Zhang, Y.; Dou, L.; Fretwurst, E.; Lindstroem, G.

    1993-12-01

    The effects of {sup 60}Co gamma irradiation on MOSCAPS and special junction diode detectors have been studied. The capacitors were used to ellicit the charge accumulation and anneal in two types of thermally grown oxides representative of those used in routine detector processing. Ion implanted, oxide passivated junction detectors having 0.25 and 1 cm{sup 2} areas and perimeter to area ratios of 1 (a square), 2 and 5 were designed and constructed to amplify the ionizing effects expected to largely affect junction edges through changes in fixed oxide charges. Detectors were exposed to over 4 Mrad and showed clear increases in leakage current in proportion to the junction edge length. Annealing schedules were determined to provide a continuous response to incremental irradiations and subsequent room temperature anneals of leakage current. Besides an increase in gate threshold, little effect on the C(V) response was found. PISCES simulation of the edge fields using different fixed oxide charge revealed regions of very high lateral fields near the junction edges for fixed charges in the 2 {times} 10{sup 12}/cm{sup 2} range expected from the capacitor studies which could be responsible for the observed leakage currents.

  3. Construction of an ionization chamber for the measurement of dose of low energy x-rays

    SciTech Connect

    Perez, Y. B. Alcantara; Jimenez, F. J. Ramirez

    2008-08-11

    We designed and constructed the prototype of an ionization chamber to measure the dose of an X-ray tube with Molybdenum anode. This X-ray tube is located in the Physics department at CINVESTAV and is used for medical physics purposes in the imaging area. The ionization chamber is designed to measure doses on biological samples exposed to X-rays and will be applied in radiation protection studies.

  4. Ionization Cross Sections and Dissociation Channels of DNA Bases by Electron Collisions

    NASA Technical Reports Server (NTRS)

    Huo, Winifred M.; Dateo, Christopher E.; Fletcher, Graham D.

    2004-01-01

    Free secondary electrons are the most abundant secondary species in ionizing radiation. Their role in DNA damage, both direct and indirect, is an active area of research. While indirect damage by free radicals, particularly by the hydroxyl radical generated by electron collision with water. is relatively well studied, damage by direct electron collision with DNA is less well understood. Only recently Boudaiffa et al. demonstrated that electrons at energies well below ionization thresholds can induce substantial yields of single- and double-strand breaks in DNA by a resonant, dissociative attachment process. This study attracted renewed interest in electron collisions with DNA, especially in the low energy region. At higher energies ionization becomes important. While Monte Carlo track simulations of radiation damage always include ionization, the probability of dissociative ionization, i.e., simultaneous ionization and dissociation, is ignored. Just like dissociative attachment, dissociative ionization may be an important contributor to double-strand breaks since the radicals and ions produced by dissociative ionization, located in the vicinity of the DNA coil, can readily interact with other parts of the DNA. Using the improved binary-encounter dipole (iBED) formulation, we calculated the ionization cross sections of the four DNA bases, adenine, cytosine, guanine, and thymine, by electrons at energies from threshold to 1 KeV. The present calculation gives cross sections approximately 20% lower than the results by Bemhardt and Paretzke using the Deutsch-Mark and Binary-Encounter-Bethe (BEB) formalisms. The difference is most likely due to the lack of a shielding term in the dipole potential used in the Deutsch-Mark and BEB formalisms. The dissociation channels of ionization for the bases are currently being studied.

  5. Ionization Cross Sections and Dissociation Channels of DNA Bases by Electron Collisions

    NASA Technical Reports Server (NTRS)

    Huo, Winifred M.; Dateo, Christopher E.; Fletcher, Graham D.

    2004-01-01

    Free secondary electrons are the most abundant secondary species in ionizing radiation. Their role in DNA damage, both direct and indirect, is an active area of research. While indirect damage by free radicals, particularly by the hydroxyl radical generated by electron collision with water. is relatively well studied, damage by direct electron collision with DNA is less well understood. Only recently Boudaiffa et al. demonstrated that electrons at energies well below ionization thresholds can induce substantial yields of single- and double-strand breaks in DNA by a resonant, dissociative attachment process. This study attracted renewed interest in electron collisions with DNA, especially in the low energy region. At higher energies ionization becomes important. While Monte Carlo track simulations of radiation damage always include ionization, the probability of dissociative ionization, i.e., simultaneous ionization and dissociation, is ignored. Just like dissociative attachment, dissociative ionization may be an important contributor to double-strand breaks since the radicals and ions produced by dissociative ionization, located in the vicinity of the DNA coil, can readily interact with other parts of the DNA. Using the improved binary-encounter dipole (iBED) formulation, we calculated the ionization cross sections of the four DNA bases, adenine, cytosine, guanine, and thymine, by electrons at energies from threshold to 1 KeV. The present calculation gives cross sections approximately 20% lower than the results by Bemhardt and Paretzke using the Deutsch-Mark and Binary-Encounter-Bethe (BEB) formalisms. The difference is most likely due to the lack of a shielding term in the dipole potential used in the Deutsch-Mark and BEB formalisms. The dissociation channels of ionization for the bases are currently being studied.

  6. Current-voltage characteristic of parallel-plane ionization chamber with inhomogeneous ionization

    NASA Astrophysics Data System (ADS)

    Stoyanov, D. G.

    2007-08-01

    The balances of particles and charges in the volume of parallel-plane ionization chamber are considered. Differential equations describing the distribution of current densities in the chamber volume are obtained. As a result of the differential equations solution an analytical form of the current-voltage characteristic of parallel-plane ionization chamber with inhomogeneous ionization in the volume is obtained.

  7. Towards a Carbon Nanotube Ionization Source for Planetary Atmosphere Exploration

    NASA Astrophysics Data System (ADS)

    Oza, A. V.; Leblanc, F.; Berthelier, J. J.; Becker, J.; Coulomb, R.; Gilbert, P.; Hong, N. T.; Lee, S.; Vettier, L.

    2015-12-01

    The characterization of planetary exospheres today, relies on the development of a highly efficient ionization source, due to the scant neutral molecules (n < 108 cm -3) present in diffuse planetary coronae. These tenuous atmospheres provide insight on to physical processes known to occur such as: space weathering, magneto-atmosphere interactions, as well as atmospheric escape mechanisms, all of which are being heavily investigated via current 3D Monte Carlo simulations (Turc et al. 2014, Leblanc et al. 2016 in prep) at LATMOS. Validation of these studies will rely on in-situ observations in the coming decades. Neutral detection strongly depends on electron-impact ionization which via conventional cathode-sources, such as thermal filaments (heated up to 2000 K), may only produce the target ionization essential for energy-measurements with large power consumption. Carbon nanotubes (CNTs) however are ideal low-power, cold cathodes, when subject to moderate electric fields (E ~ 1 MV / m). We present our current device, a small CNT chip, of emission area 15 mm2, emitting electrons that pass through an anode grid and subsequent electrostatic analyzer. The device currently extracts hundreds of µAmperes with applied external voltages ~ -150 Volts, approaching minimum power consumption < 0.1 Watts. The 3D modeling of field effect electrons ionizing a standard influx of neutrals is shown, using the multiphysics suite COMSOL. To better anticipate the species an ideal in-situ spacecraft equipped with such an ionization source would observe, we discuss Europa's exosphere. Europa's environment is largely shaped by the Jovian plasma sputtering the icy regolith with heavy ions and electrons (keV < E < MeV), producing predominately molecular oxygen (Johnson et al. 2002).

  8. Multiphoton ionization of uranium hexafluoride

    NASA Astrophysics Data System (ADS)

    Armstrong, D. P.; Harkins, D. A.; Compton, R. N.; Ding, D.

    1994-01-01

    Multiphoton ionization (MPI) time-of-flight mass spectroscopy (TOFMS) and photoelectron spectroscopy (PES) studies of UF6 are reported using focused light from the Nd:YAG laser fundamental (λ=1064 nm) and its harmonics (λ=532, 355, or 266 nm), as well as other wavelengths provided by a tunable dye laser. The MPI mass spectra are dominated by the singly and multiply charged uranium ions rather than by the UF+x fragment ions, even at the lowest laser power densities at which signal could be detected. In general, the doubly charged uranium ion (U2+) intensity is much greater than that of the singly charged uranium ion (U+). For the case of the tunable dye laser experiments, the Un+ (n=1-4) wavelength dependence is relatively unstructured and does not show observable resonance enhancement at known atomic uranium excitation wavelengths. The MPI-PES studies reveal only very slow electrons (≤0.5 eV) for all wavelengths investigated. The dominance of the U2+ ion, the absence or very small intensities of UF+x (x=1-3) fragments, the unstructured wavelength dependence, and the preponderance of slow electrons all indicate that mechanisms may exist other than ionization of bare U atoms following the stepwise photodissociation of F atoms from the parent molecule. The data also argue against stepwise photodissociation of UF+x (x=5,6) ions. Neither of the traditional MPI mechanisms (``neutral ladder'' or the ``ionic ladder'') are believed to adequately describe the ionization phenomena observed. We propose that the multiphoton excitation of UF6 under these experimental conditions results in a highly excited molecule, superexcited UF6**. The excitation of highly excited UF6** is proposed to be facilitated by the well known ``giant resonance,'' whose energy level lies in the range of 12-14 eV above that of ground state UF6. The highly excited molecule then primarily dissociates, via multiple channels, into Un+, UF+x, fluorine atoms, and ``slow'' electrons, although dissociation

  9. Field ionization of free helium atoms: Correlation between the kinetic energy of ionized atoms and probability of their field ionization

    NASA Astrophysics Data System (ADS)

    Piskur, J.; Borg, L.; Stupnik, A.; Leisch, M.; Ernst, W. E.; Holst, B.

    2008-05-01

    In this paper the correlation between the kinetic energy of helium atoms and the probability of field ionization is investigated by exploiting the narrow velocity distribution of supersonic molecular beams. Field ionization measurements were carried out on supersonic helium beams at 298 K and 95 K corresponding to energies of about 65 meV and 20 meV, respectively, for the individual atoms. The field ionization was performed with a tungsten tip, radius of curvature 12 nm, kept at room temperature. The ionization probability was found to increase by about a factor 10 when the beam was cooled from 298 K to 95 K. The results presented in this paper are of importance for improving the understanding of field ionization and for the development of a new detector for helium and other molecular beams.

  10. The Contribution of Field OB Stars to the Ionization of the Diffuse Ionized Gas in M33

    NASA Astrophysics Data System (ADS)

    Hoopes, Charles G.; Walterbos, René A. M.

    2000-10-01

    We present a study of the ionizing stars associated with the diffuse ionized gas (DIG) and H II regions in the nearby spiral galaxy M33. We compare our Schmidt Hα image to the far-ultraviolet (FUV, 1520 Å) image from the Ultraviolet Imaging Telescope (UIT). The Hα/FUV ratio is higher in H II regions than in the DIG, suggesting an older population of ionizing stars in the DIG. Assuming ionization equilibrium, we convert the Hα flux to the number of Lyman continuum photons NLyc. When compared to models of evolving stellar populations, the NLyc/FUV ratio in H II regions is consistent with a young burst, while the DIG ratio resembles an older burst population, or a steady state population built up by constant star formation, which is probably a more accurate description of the stellar population in the field. The UIT data is complemented with archival FUV and optical images of a small portion of the disk of M33 obtained with WFPC2 on board the Hubble Space Telescope (HST). These images overlap low- and mid-luminosity H II regions as well as DIG, so we can investigate the stellar population in these environments. Using the HST FUV and optical photometry, we assign spectral types to the stars observed in DIG and H II regions. The photometry indicates that ionizing stars are present in the DIG. We compare the predicted ionizing flux with the amount required to produce the observed Hα emission, and we find that field OB stars in the HST images can account for 40%+/-12% of the ionization of the DIG, while the stars in H II regions can provide 107%+/-26% of the Hα luminosity of the H II regions. Due to the limited coverage of the HST data, we cannot determine if stars outside the HST fields ionize some of the DIG located in the HST fields, nor can we determine if photons from stars inside the HST fields leak out of the area covered by the HST fields. We do not find any correlation between leakage of ionizing photons and Hα luminosity for the H II regions in our HST

  11. Ionization in nearby interstellar gas

    NASA Technical Reports Server (NTRS)

    Frisch, P. C.; Welty, D. E.; York, D. G.; Fowler, J. R.

    1990-01-01

    Due to dielectric recombination, neutral magnesium represents an important tracer for the warm low-density gas around the solar system. New Mg I 2852 absorption-line data from IUE are presented, including detections in a few stars within 40 pc of the sun. The absence of detectable Mg I in Alpha CMa and other stars sets limits on the combined size and electron density of the interstellar cloud which gives rise to the local interstellar wind. For a cloud radius greater than 1 pc and density of 0.1/cu cm, the local cloud has a low fractional ionization, n(e)/n(tot) less than 0.05, if magnesium is undepleted, equilibrium conditions prevail, the cloud temperature is 11,750 K, and 80 percent of the magnesium in the sightline is Mg II.

  12. Ionization tube simmer current circuit

    DOEpatents

    Steinkraus, Jr., Robert F.

    1994-01-01

    A highly efficient flash lamp simmer current circuit utilizes a fifty percent duty cycle square wave pulse generator to pass a current over a current limiting inductor to a full wave rectifier. The DC output of the rectifier is then passed over a voltage smoothing capacitor through a reverse current blocking diode to a flash lamp tube to sustain ionization in the tube between discharges via a small simmer current. An alternate embodiment of the circuit combines the pulse generator and inductor in the form of an FET off line square wave generator with an impedance limited step up output transformer which is then applied to the full wave rectifier as before to yield a similar simmer current.

  13. Electrospray Ionization on Solid Substrates

    PubMed Central

    So, Pui-Kin; Hu, Bin; Yao, Zhong-Ping

    2014-01-01

    Development of electrospray ionization on solid substrates (solid-substrate ESI) avoids the clogging problem encountered in conventional capillary-based ESI, allows more convenient sampling and permits new applications. So far, solid-substrate ESI with various materials, e.g., metals, paper, wood, fibers and biological tissue, has been developed, and applications ranging from analysis of pure compounds to complex mixtures as well as in vivo study were demonstrated. Particularly, the capability of solid-substrate ESI in direct analysis of complex samples, e.g., biological fluids and foods, has significantly facilitated mass spectrometric analysis in real-life applications and led to increasingly important roles of these techniques nowadays. In this review, various solid-substrate ESI techniques and their applications are summarized and the prospects in this field are discussed. PMID:26819900

  14. Ionization tube simmer current circuit

    DOEpatents

    Steinkraus, R.F. Jr.

    1994-12-13

    A highly efficient flash lamp simmer current circuit utilizes a fifty percent duty cycle square wave pulse generator to pass a current over a current limiting inductor to a full wave rectifier. The DC output of the rectifier is then passed over a voltage smoothing capacitor through a reverse current blocking diode to a flash lamp tube to sustain ionization in the tube between discharges via a small simmer current. An alternate embodiment of the circuit combines the pulse generator and inductor in the form of an FET off line square wave generator with an impedance limited step up output transformer which is then applied to the full wave rectifier as before to yield a similar simmer current. 6 figures.

  15. Benchmarking Ionizing Space Environment Models

    NASA Astrophysics Data System (ADS)

    Bourdarie, S.; Inguimbert, C.; Standarovski, D.; Vaillé, J.-R.; Sicard-Piet, A.; Falguere, D.; Ecoffet, R.; Poivey, C.; Lorfèvre, E.

    2017-08-01

    In-flight feedback data are collected, such as displacement damage doses, ionizing doses, and cumulated Single Event upset (SEU) on board various space vehicles and are compared to predictions performed with: 1) proton measurements performed with spectrometers data on board the same spacecraft if any and 2) protons spectrum predicted by the legacy AP8min model and the AP9 and Onera Proton Altitude Low models. When an accurate representation of the 3-D spacecraft shielding as well as appropriate ground calibrations are considered in the calculations, such comparisons provide powerful metrics to investigate engineering model accuracy. To describe >30 MeV trapped protons fluxes, the AP8 min model is found to provide closer predictions to observations than AP9 V1.30.001 (mean and perturbed mean).

  16. Large area mass analyzer

    NASA Astrophysics Data System (ADS)

    Rachev, Mikhail; Srama, Ralf; Srowig, Andre; Grün, Eberhard

    2004-12-01

    A new time-of-flight spectrometer for the chemical analysis of cosmic dust particles in space has been simulated by Simion 7.0. The instrument is based upon impact ionization. This method is a reliable method for in situ dust detection and is well established. Instruments using the impact ionization flew on board of Helios and Galileo and are still in operation on board of the Ulysses and Cassini-Huygens missions. The new instrument has a large sensitive area of 0.1 m2 in order to achieve a significant number of measurements. The mass resolution M/ΔM>100 and the mass range covers the most relevant elements expected in cosmic dust. The instrument has a reflectron configuration which increases the mass resolution. Most of the ions released during the impact are focused to the detector. The ion detector consists of a large area ion-to-electron converter, an electron reflectron and a microchannel plate detector.

  17. Miniature Oxidizer Ionizer for a Fuel Cell

    NASA Technical Reports Server (NTRS)

    Hartley, Frank

    2006-01-01

    A proposed miniature device for ionizing the oxygen (or other oxidizing gas) in a fuel cell would consist mostly of a membrane ionizer using the same principles as those of the device described in the earlier article, Miniature Bipolar Electrostatic Ion Thruster (NPO-21057). The oxidizing gas would be completely ionized upon passage through the holes in the membrane ionizer. The resulting positively charged atoms or molecules of oxidizing gas could then, under the influence of the fringe fields of the ionizer, move toward the fuel-cell cathode that would be part of a membrane/electrode assembly comprising the cathode, a solid-electrolyte membrane, and an anode. The electro-oxidized state of the oxidizer atoms and molecules would enhance transfer of them through the cathode, thereby reducing the partial pressure of the oxidizer gas between the ionizer and the fuel-cell cathode, thereby, in turn, causing further inflow of oxidizer gas through the holes in the membrane ionizer. Optionally the ionizer could be maintained at a positive electric potential with respect to the cathode, in which case the resulting electric field would accelerate the ions toward the cathode.

  18. Ultrafast ionization and fragmentation of molecular silane

    SciTech Connect

    Sayres, Scott G.; Ross, Matt W.; Castleman, A. W. Jr.

    2010-09-15

    The ionization and fragmentation of molecular silane is examined here with laser intensities ranging between 7x10{sup 12} and 1x10{sup 15} W/cm{sup 2} at 624 nm. The ionization potential of silane determined using both multiphoton ionization (MPI) and tunneling ionization (TI) models agrees with the vertical ionization potential of the molecule. In addition, the application of the tunneling ionization model is extended here to the fragments of silane to determine their appearance potentials. MPI values for SiH{sub 3}{sup +}, SiH{sub 2}{sup +}, SiH{sup +}, Si{sup +}, as well as H{sub 2}{sup +} and H{sup +} are consistent with vertical potentials, whereas the TI measurements are found to be in accord with adiabatic potentials. The tunneling appearance potentials observed for the fragments H{sub 2}{sup +} and H{sup +} are lower than reported for other techniques. In fact, the appearance potential measurements for these species resulting from silane are lower than their ionization potentials. The fragmentation rate of silane is determined to be nearly 20 times larger than the ionization rate. The main precursor for producing amorphous silicon (a-Si:H) thin films, SiH{sub 3}{sup +} is the dominant fragmentation product making up roughly a third of the total ion yield, a substantial increase from other techniques.

  19. Forensic applications of ambient ionization mass spectrometry.

    PubMed

    Ifa, Demian R; Jackson, Ayanna U; Paglia, Giuseppe; Cooks, R Graham

    2009-08-01

    This review highlights and critically assesses forensic applications in the developing field of ambient ionization mass spectrometry. Ambient ionization methods permit the ionization of samples outside the mass spectrometer in the ordinary atmosphere, with minimal sample preparation. Several ambient ionization methods have been created since 2004 and they utilize different mechanisms to create ions for mass-spectrometric analysis. Forensic applications of these techniques--to the analysis of toxic industrial compounds, chemical warfare agents, illicit drugs and formulations, explosives, foodstuff, inks, fingerprints, and skin--are reviewed. The minimal sample pretreatment needed is illustrated with examples of analysis from complex matrices (e.g., food) on various substrates (e.g., paper). The low limits of detection achieved by most of the ambient ionization methods for compounds of forensic interest readily offer qualitative confirmation of chemical identity; in some cases quantitative data are also available. The forensic applications of ambient ionization methods are a growing research field and there are still many types of applications which remain to be explored, particularly those involving on-site analysis. Aspects of ambient ionization currently undergoing rapid development include molecular imaging and increased detection specificity through simultaneous chemical reaction and ionization by addition of appropriate chemical reagents.

  20. Astatine and Yttrium Resonant Ionization Laser Spectroscopy

    NASA Astrophysics Data System (ADS)

    Teigelhoefer, Andrea

    Providing intense, contamination-free beams of rare isotopes to experiments is a challenging task. At isotope separator on-line facilities such as ISAC at TRIUMF, the choice of production target and ion source are key to the successful beam delivery. Due to their element-selectivity, high efficiency and versatility, resonant ionization laser ion sources (RILIS) gain increasingly in importance. The spectroscopic data available are typically incomplete in the region of excited- and autoionizing atomic states. In order to find the most efficient ionization scheme for a particular element, further spectroscopy is often required. The development of efficient laser resonant ionization schemes for yttrium and astatine is presented in this thesis. For yttrium, two ionization schemes with comparable relative intensities were found. Since for astatine, only two transitions were known, the focus was to provide data on atomic energy levels using resonance ionization spectroscopy. Altogether 41 previously unknown astatine energy levels were found.

  1. Inner-orbital ionization of iodine

    NASA Astrophysics Data System (ADS)

    Gibson, George; Smith, Dale; Tagliamonti, Vincent; Dragan, James

    2016-05-01

    Many coincidence techniques exist to study multiple ionization of molecules by strong laser fields. However, the first ionization step is critical in many experiments, although it is more difficult to obtain information about this initial step. We studied the single electron ionization of I2, as it presents interesting opportunities in that it is heavy and does not expand significantly during the laser pulse. Moreover, there are several distinct low-lying valence orbitals from which the electron may be removed. Most importantly, the kinetic energy release of the I+ + I dissociation channel can be measured and should correspond to well-known valence levels and separated atom limits. As it turns out, we must invoke deep valence orbits, built from the 5s electrons, to explain our data. Ionization from deep orbitals may be possible, as they have a smaller critical internuclear separation for enhanced ionization. We would like to acknowledge support from the NSF under Grant No. PHY-1306845.

  2. Improved Imaging Resolution in Desorption Electrospray Ionization Mass Spectrometry

    SciTech Connect

    Kertesz, Vilmos; Van Berkel, Gary J

    2008-01-01

    Imaging resolution of desorption electrospray ionization mass spectrometry (DESI-MS) was investigated using printed patterns on paper and thin-layer chromatography (TLC) plate surfaces. Resolution approaching 40 m was achieved with a typical DESI-MS setup, which is approximately 5 times better than the best resolution reported previously. This improvement was accomplished with careful control of operational parameters (particularly spray tip-to-surface distance, solvent flow rate, and spacing of lane scans). Also, an appropriately strong analyte/surface interaction and uniform surface texture on the size scale no larger that the desired imaging resolution were required to achieve this resolution. Overall, conditions providing the smallest possible effective desorption/ionization area in the DESI impact plume region and minimizing the analyte redistribution on the surface during analysis led to the improved DESI-MS imaging resolution.

  3. Electron impact ionization and multiphoton ionization of doped superfluid helium droplets: A comparison.

    PubMed

    He, Yunteng; Zhang, Jie; Kong, Wei

    2016-02-28

    We compare characteristics of electron impact ionization (EI) and multiphoton ionization (MPI) of doped superfluid helium droplets using the same droplet source. Selected dopant ion fragments from the two ionization schemes demonstrate different dependence on the doping pressure, which could be attributed to the different ionization mechanisms. While EI directly ionizes helium atoms in a droplet therefore has higher yields for bigger droplets (within a limited size range), MPI is insensitive to the helium in a droplet and is only dependent on the number of dopant molecules. The optimal timing of the ionization pulse also varies with the doping pressure, implying a velocity slip among different sized droplets. Calculations of the doping statistics and ionization probabilities qualitatively agree with the experimental data. Our results offer a word of caution in interpreting the pressure and timing dependence of superfluid helium droplets, and we also devise a scheme in achieving a high degree of doping while limiting the contribution of dopant clusters.

  4. Electron impact ionization and multiphoton ionization of doped superfluid helium droplets: A comparison

    PubMed Central

    2016-01-01

    We compare characteristics of electron impact ionization (EI) and multiphoton ionization (MPI) of doped superfluid helium droplets using the same droplet source. Selected dopant ion fragments from the two ionization schemes demonstrate different dependence on the doping pressure, which could be attributed to the different ionization mechanisms. While EI directly ionizes helium atoms in a droplet therefore has higher yields for bigger droplets (within a limited size range), MPI is insensitive to the helium in a droplet and is only dependent on the number of dopant molecules. The optimal timing of the ionization pulse also varies with the doping pressure, implying a velocity slip among different sized droplets. Calculations of the doping statistics and ionization probabilities qualitatively agree with the experimental data. Our results offer a word of caution in interpreting the pressure and timing dependence of superfluid helium droplets, and we also devise a scheme in achieving a high degree of doping while limiting the contribution of dopant clusters. PMID:26931697

  5. CHAMBER - IONIZATION - EXPERIMENT - GEMINI-TITAN (GT)-6 EQUIPMENT - CAPE

    NASA Image and Video Library

    1965-12-10

    S65-61788 (For release: 11 Dec. 1965) --- Close-up view of equipment which will be used in the D-8 (Radiation in Spacecraft) experiment on the National Aeronautics and Space Administration's Gemini-6 spaceflight. This experiment is designed to make highly accurate measurements of the absorbed dose rate of radiation which penetrates the Gemini spacecraft, and determine the spatial distribution of dose levels inside the spacecraft particularly in the crew area. This is experimentation of the U.S. Air Force Weapons Laboratory, Kirtland AFB, N.M. LOWER LEFT: The second ionization chamber, this one is unshielded. This chamber can be removed from its bracket by the astronaut who will periodically take measurements at various locations in the spacecraft. Nearby is Passive Dosimeter Unit which is one of five small packets each containing a standard pocket ionization chamber, gamma electron sensitive film, glass needles and thermo luminescent dosimeters which are mounted at various locations in the cabin. UPPER LEFT: Photo illustrates how ionization chamber can be removed from bracket for measurements. LOWER RIGHT: Shield of bulb-shaped chamber will be removed (shown in photo) as the spacecraft passes through the South Atlantic anomaly, the area where the radiation belt dips closest to Earth's surface. UPPER RIGHT: Dome-shaped object is shield covering one of two Tissue Equivalent Ionization Chambers (sensors) which will read out continuously the instantaneous rate at which dose is delivered during the flight. This chamber is mounted permanently. The information will be recorded aboard the spacecraft, and will also be received directly by ground stations. This chamber is shielded to simulate the amount of radiation the crew members are receiving beneath their skin. Photo credit: NASA or National Aeronautics and Space Administration

  6. Ionizing radiation and breast cancer in men (United States).

    PubMed

    Thomas, D B; Rosenblatt, K; Jimenez, L M; McTiernan, A; Stalsberg, H; Stemhagen, A; Thompson, W D; Curnen, M G; Satariano, W; Austin, D F

    1994-01-01

    The purposes of this study were to determine whether exposure of the vestigial male breast to ionizing radiation is associated with an increase in risk of breast cancer and, if so, to determine whether the apparent effects on risk in men are similar to those reported for women. A population-based case-control study of breast cancer in men was conducted in 10 geographic areas of the United States. Information on possible prior exposure to ionizing radiation, and on other potential risk factors for breast cancer, was obtained from personal interviews of 227 cases and 300 controls who were recruited from October 1983 to September 1986. Evidence from this study that ionizing radiation can cause breast cancer in men includes: a modest trend of increasing risk with frequency of chest X-rays; an increase in risk in men with three or more radiographic examinations, especially if received prior to 1963; and an increase in risk in men who received X-ray treatments to the chest and adjacent body areas. Risk was increased only from 20 to 35 years after initial exposure from either radiographic examinations or X-ray treatments, and declined after three to four decades since last exposure, suggesting a wave of increased risk of finite duration following exposure. The doses of radiation received could not be estimated precisely, but those from diagnostic procedures were likely similar to those received by prepubertal females in prior studies, and the results of those and the present investigation are compatible. The carcinogenic effects of ionizing radiation may be similar in the male and prepubertal female breast.

  7. Non-Ionizing Radiation Used in Microwave Ovens

    MedlinePlus

    ... Ionizing Radiation Used in Microwave Ovens Non-Ionizing Radiation Used in Microwave Ovens Explore the interactive, virtual ... do Where to learn more About Non-Ionizing Radiation Used in Microwave Ovens Microwave Oven. Microwave ovens ...

  8. Ionization Cooling using Parametric Resonances

    SciTech Connect

    Johnson, Rolland P.

    2008-06-07

    Ionization Cooling using Parametric Resonances was an SBIR project begun in July 2004 and ended in January 2008 with Muons, Inc., (Dr. Rolland Johnson, PI), and Thomas Jefferson National Accelerator Facility (JLab) (Dr. Yaroslav Derbenev, Subcontract PI). The project was to develop the theory and simulations of Parametric-resonance Ionization Cooling (PIC) so that it could be used to provide the extra transverse cooling needed for muon colliders in order to relax the requirements on the proton driver, reduce the site boundary radiation, and provide a better environment for experiments. During the course of the project, the theoretical understanding of PIC was developed and a final exposition is ready for publication. Workshops were sponsored by Muons, Inc. in May and September of 2007 that were devoted to the PIC technique. One outcome of the workshops was the interesting and somewhat unexpected realization that the beam emittances using the PIC technique can get small enough that space charge forces can be important. A parallel effort to develop our G4beamline simulation program to include space charge effects was initiated to address this problem. A method of compensating for chromatic aberrations by employing synchrotron motion was developed and simulated. A method of compensating for spherical aberrations using beamline symmetry was also developed and simulated. Different optics designs have been developed using the OptiM program in preparation for applying our G4beamline simulation program, which contains all the power of the Geant4 toolkit. However, no PIC channel design that has been developed has had the desired cooling performance when subjected to the complete G4beamline simulation program. This is believed to be the consequence of the difficulties of correcting the aberrations associated with the naturally large beam angles and beam sizes of the PIC method that are exacerbated by the fringe fields of the rather complicated channel designs that have been

  9. Laser resonance ionization spectroscopy of antimony

    NASA Astrophysics Data System (ADS)

    Li, R.; Lassen, J.; Ruczkowski, J.; Teigelhöfer, A.; Bricault, P.

    2017-02-01

    The resonant ionization laser ion source is an element selective, efficient and versatile ion source to generate radioactive ion beams at on-line mass separator facilities. For some elements with complex atomic structures and incomplete spectroscopic data, laser spectroscopic investigations are required for ionization scheme development. Laser resonance ionization spectroscopy using Ti:Sa lasers has been performed on antimony (Sb) at TRIUMF's off-line laser ion source test stand. Laser light of 230.217 nm (vacuum wavelength) as the first excitation step and light from a frequency-doubled Nd:YVO4 laser (532 nm) as the nonresonant ionization step allowed to search for suitable second excitation steps by continuous wavelength scans from 720 nm to 920 nm across the wavelength tuning range of a grating-tuned Ti:Sa laser. Upon the identification of efficient SES, the third excitation steps for resonance ionization were investigated by laser scans across Rydberg states, the ionization potential and autoionizing states. One Rydberg state and six AI states were found to be well suitable for efficient resonance ionization.

  10. Laser-induced ionization of Na vapor

    SciTech Connect

    Wu, R.C.Y.; Judge, D.L.; Roussel, F.; Carre, B.; Breger, P.; Spiess, G.

    1982-01-01

    The production of Na/sub 2//sup +/ ions by off-resonant laser excitation in the 5800-6200A region mainly results from two-photon absorption by the Na/sub 2/ molecule to highly excited gerade states followed by (a) direct ionization by absorbing a third photon or (b) coupling to the molecular Na/sub 2/ D/sup 1/PI..mu.. Rydberg state which is subsequently ionized by absorbing a third photon. This mechanism, i.e., a two-photon resonance three photon ionization process, explains a recent experimental observation of Roussel et al. It is suggested that the very same mechanism is also responsible for a similar observation reported by Polak-Dingels et al in their work using two crossed Na beams. In the latter two studies the laser-induced associative ionization processes were reported to be responsible for producing the Na/sub 2//sup +/ ion. From the ratio of molecular to atomic concentration in the crossed beam experiment of Polak-Dingels et al we estimate that the cross section for producing Na/sub 2//sup +/ through laser-induced associative ionization is at least four orders of magnitude smaller than ionization through the two-photon resonance three photon ionization process in Na/sub 2/ molecules.

  11. Laser-induced ionization of Na vapor

    NASA Astrophysics Data System (ADS)

    Wu, C. Y. Robert; Judge, D. L.; Roussel, F.; Carré, B.; Breger, P.; Spiess, G.

    1982-09-01

    The production of Na2+ ions by off-resonant laser excitation in the 5800-6200Å region mainly results from two-photon absorption by the Na2 molecule to highly excited gerade states followed by (a) direct ionization by absorbing a third photon or (b) coupling to the molecular Na2 D1Πu Rydberg state which is subsequently ionized by absorbing a third photon. This mechanism, i.e., a two-photon resonance three photon ionization process, explains a recent experimental observation of Roussel et al. It is suggested that the very same mechanism is also responsible for a similar observation reported by Polak-Dingels et al in their work using two crossed Na beams. In the latter two studies the laser-induced associative ionization processes were reported to be responsible for producing the Na2+ ion. From the ratio of molecular to atomic concentration in the crossed beam experiment of Polak-Dingels et al. we estimate that the cross section for producing Na2+ through laser-induced associative ionization is at least four orders of magnitude smaller than ionization through the two-photon resonance three photon ionization process in Na2 molecules.

  12. Sub-cycle dynamics of multiphoton ionization

    NASA Astrophysics Data System (ADS)

    Telnov, Dmitry A.; Nasiri Avanaki, K.; Chu, Shih-I.

    2014-05-01

    Sub-cycle oscillatory structures are revealed in calculated time-dependent multiphoton ionization rates. Both atomic and molecular targets manifest multiple ionization bursts per one optical cycle of the laser field. Using the accurate and efficient time-dependent generalized pseudospectral method to solve the time-dependent Schrödinger equation, we have performed calculations on H, He+, H2+,and HHe2+, for the laser fields with several intensities and wavelengths in the near-infrared range (750 nm to 1064 nm). The sub-cycle structures appear a universal feature of multiphoton ionization and become well pronounced for sufficiently strong laser fields depending on the target atom or molecule. Analysis of the electron density distributions on the sub-femtosecond time scale shows several time moments per optical cycle (not necessarily corresponding to the peak values of the laser field) when significant portions of the electron density move away from the nucleus giving rise to the bursts in the ionization rate. The nature of the phenomenon can be related to ionization through different pathways, including direct ionization as well as population of the excited states by the laser field with subsequent ionization at later times. This work is partially supported by DOE.

  13. Re-ionization and decaying dark matter

    NASA Technical Reports Server (NTRS)

    Dodelson, Scott; Jubas, Jay M.

    1991-01-01

    Gunn-Peterson tests suggest that the Universe was reionized after the standard recombination epoch. A systematic treatment is presented of the ionization process by deriving the Boltzmann equations appropriate to this regime. A compact solution for the photon spectrum is found in terms of the ionization ratio. These equations are then solved numerically for the Decaying Dark Matter scenario, wherein neutrinos with mass of order 30 eV radiatively decay producing photons which ionize the intergalactic medium. It was found that the neutrino mass and lifetime are severely constrained by Gunn-Peterson tests, observations of the diffuse photon spectrum in the ultraviolet regime, and the Hubble parameter.

  14. Charged-Particle Impact Ionization of Atoms

    SciTech Connect

    Bartschat, Klaus; Guan Xiaoxu

    2008-08-08

    We have developed a hybrid method to treat charged-particle impact ionization of complex atoms and ions. The essential idea is to describe the interaction between a fast projectile and the target perturbatively, up to second order, while the initial bound state and the ejected-electron--residual-ion interaction can be handled via a convergent R-matrix with pseudo-states (close-coupling) expansion. Example results for ionization of the heavy noble gases (Ne-Xe) by positron and electron impact are presented. The general scheme for a distorted-wave treatment of ionization by heavy-particle impact is described.

  15. Ionization of excited xenon atoms by electrons

    NASA Astrophysics Data System (ADS)

    Erwin, Daniel A.; Kunc, Joseph A.

    2004-08-01

    Measured cross sections for electron-impact ionization of excited Xe atoms are not presently available. Therefore, we combine in this work the formalisms of the binary encounter approximation and Sommerfeld’s quantization of atomic orbits and derive from first-principles cross sections for ionization of excited atoms by electrons of low and moderate energies (up to a few hundred eV ). The approach of this work can be used to calculate the cross sections for electron-impact ionization of excited atoms and atomic ions other than xenon.

  16. Epicyclic Twin-Helix Ionization Cooling Simulations

    SciTech Connect

    Vasiliy Morozov, Yaroslav Derbenev, A. Afanaciev, R.P. Johnson

    2011-04-01

    Parametric-resonance Ionization Cooling (PIC) is proposed as the final 6D cooling stage of a highluminosity muon collider. For the implementation of PIC, we earlier developed an epicyclic twin-helix channel with correlated behavior of the horizontal and vertical betatron motions and dispersion. We now insert absorber plates with short energy-recovering units located next to them at the appropriate locations in the twin-helix channel. We first demonstrate conventional ionization cooling in such a system with the optics uncorrelated. We then adjust the correlated optics state and induce a parametric resonance to study ionization cooling under the resonant condition.

  17. Probing Angular Correlations in Sequential Double Ionization

    SciTech Connect

    Fleischer, A.; Woerner, H. J.; Arissian, L.; Liu, L. R.; Meckel, M.; Rippert, A.; Doerner, R.; Villeneuve, D. M.; Corkum, P. B.; Staudte, A.

    2011-09-09

    We study electron correlation in sequential double ionization of noble gas atoms and HCl in intense, femtosecond laser pulses. We measure the photoelectron angular distributions of Ne{sup +} relative to the first electron in a pump-probe experiment with 8 fs, 800 nm, circularly polarized laser pulses at a peak intensity of a few 10{sup 15} W/cm{sup 2}. Using a linear-linear pump-probe setup, we further study He, Ar, and HCl. We find a clear angular correlation between the two ionization steps in the sequential double ionization intensity regime.

  18. Non-equilibrium ionized blast wave

    NASA Technical Reports Server (NTRS)

    Wu, S. T.

    1974-01-01

    The structure of a cylindrical blast wave with ionization at non-LTE conditions was calculated using equations previously developed by Wu and Fu (1970). The degree of ionization was predicted by a modified Saha equation. Temperature profiles show that the temperature at non-LTE conditions is lower than at LTE near the shock front. This corresponds to a higher degree of ionization for the non-LTE limit, which indicates that the neutral gas absorption is much more efficient at non-LTE than at the LTE limit. The decaying velocity under non-LTE is approximately 15% less than under LTE.

  19. Ionization and Triggered Star Formation

    NASA Astrophysics Data System (ADS)

    Gritschneder, M.; Lin, D. N. C.; Murray, S. D.; Burkert, A.

    2011-12-01

    We perform a set of high resolution simulations on the impact of the UV-radiation of massive stars on the turbulent interstellar medium with the tree-SPH code iVINE. This parameter study includes different levels and driving scales of the turbulence, different ionizing flux as well as different temperatures and densities of the cold gas. We find a clear correlation between the initial state of the turbulent cloud and the final morphology and physical properties of the structures adjacent to the HII region. From the simulations we are able to derive a criterion for the formation of pillar-like structures and thus the formation of cores and stars. Gravitational collapse occurs regularly on the tips of the structures. We also derive column densities and velocity profiles of our simulations and find these to be in very good agreement with the observations of trunks and cores. In addition, we investigate the further evolution of the pillars once the massive star explodes. This leads to a supernova triggered scenario for the formation of our Solar System.

  20. Ionized Carbon Atoms in Orion

    NASA Image and Video Library

    2016-10-12

    The dusty side of the Sword of Orion is illuminated in this striking infrared image from the European Space Agency's Hershel Space Observatory. This immense nebula is the closest large region of star formation, situated about 1,500 light years away in the constellation of Orion. The parts that are easily observed in visible light, known alternatively as the Orion Nebula or Messier 42, correspond to the light blue regions. This is the glow from the warmest dust, illuminated by clusters of hot stars that have only recently been born in this chaotic region. The red spine of material running from corner to corner reveals colder, denser filaments of dust and gas that are scattered throughout the Orion nebula. In visible light this would be a dark, opaque feature, hiding the reservoir of material from which stars have recently formed and will continue to form in the future. Herschel data from the PACS instrument observations, at wavelengths of 100 and 160 microns, is displayed in blue and green, respectively, while SPIRE 250-micron data is shown in red. Within the inset image, the emission from ionized carbon atoms (C+), overlaid in yellow, was isolated and mapped out from spectrographic data obtained by the HIFI instrument. http://photojournal.jpl.nasa.gov/catalog/PIA21073

  1. Ionizing radiation and hematopoietic malignancies

    PubMed Central

    Fleenor, Courtney J; Marusyk, Andriy

    2010-01-01

    Somatic evolution, which underlies tumor progression, is driven by two essential components: (1) diversification of phenotypes through heritable mutations and epigenetic changes and (2) selection for mutant clones which possess higher fitness. Exposure to ionizing radiation (IR) is highly associated with increased risk of carcinogenesis. This link is traditionally attributed to causation of oncogenic mutations through the mutagenic effects of irradiation. On the other hand, potential effects of irradiation on altering fitness and increasing selection for mutant clones are frequently ignored. Recent studies bring the effects of irradiation on fitness and selection into focus, demonstrating that IR exposure results in stable reductions in the fitness of hematopoietic stem and progenitor cell populations. These reductions of fitness are associated with alteration of the adaptive landscape, increasing the selective advantages conferred by certain oncogenic mutations. Therefore, the link between irradiation and carcinogenesis might be more complex than traditionally appreciated: while mutagenic effects of irradiation should increase the probability of occurrence of oncogenic mutations, IR can also work as a tumor promoter, increasing the selective expansion of clones bearing mutations which become advantageous in the irradiation-altered environment, such as activated mutations in Notch1 or disrupting mutations in p53. PMID:20676038

  2. Ionizing radiation and heart risks.

    PubMed

    Bhattacharya, Souparno; Asaithamby, Aroumougame

    2016-10-01

    Cardiovascular disease and cancer are the two leading causes of morbidity and mortality worldwide. As advancements in radiation therapy (RT) have significantly increased the number of cancer survivors, the risk of radiation-induced cardiovascular disease (RICD) in this group is a growing concern. Recent epidemiological data suggest that accidental or occupational exposure to low dose radiation, in addition to therapeutic ionizing radiation, can result in cardiovascular complications. The progression of radiation-induced cardiotoxicity often takes years to manifest but is also multifaceted, as the heart may be affected by a variety of pathologies. The risk of cardiovascular disease development in RT cancer survivors has been known for 40 years and several risk factors have been identified in the last two decades. However, most of the early work focused on clinical symptoms and manifestations, rather than understanding cellular processes regulating homeostatic processes of the cardiovascular system in response to radiation. Recent studies have suggested that a different approach may be needed to refute the risk of cardiovascular disease following radiation exposure. In this review, we will focus on how different radiation types and doses may induce cardiovascular complications, highlighting clinical manifestations and the mechanisms involved in the pathophysiology of radiation-induced cardiotoxicity. We will finally discuss how current and future research on heart development and homeostasis can help reduce the incidence of RICD.

  3. Magnetohydrodynamic turbulence and turbulent dynamo in partially ionized plasma

    NASA Astrophysics Data System (ADS)

    Xu, Siyao; Lazarian, A.

    2017-06-01

    Astrophysical fluids are turbulent, magnetized, and frequently partially ionized. As an example of astrophysical turbulence, the interstellar turbulence extends over a remarkably large range of spatial scales and participates in key astrophysical processes happening on different ranges of scales. Significant progress has been achieved in the understanding of the magnetohydrodynamic (MHD) turbulence since the turn of the century, and this enables us to better describe turbulence in magnetized and partially ionized plasmas. In fact, the modern revolutionized picture of MHD turbulence physics facilitates the development of various theoretical domains, including the damping process for dissipating MHD turbulence and the dynamo process for generating MHD turbulence with many important astrophysical implications. In this paper, we review some important findings from our recent theoretical works to demonstrate the interconnection between the properties of MHD turbulence and those of turbulent dynamo in a partially ionized gas. We also briefly exemplify some new tentative studies on how the revised basic processes influence the associated outstanding astrophysical problems in areas such as magnetic reconnection, cosmic ray scattering, and magnetic field amplification in both the early and present-day universe.

  4. Matrix Assisted Ionization Vacuum (MAIV), a New Ionization Method for Biological Materials Analysis Using Mass Spectrometry*

    PubMed Central

    Inutan, Ellen D.; Trimpin, Sarah

    2013-01-01

    The introduction of electrospray ionization (ESI) and matrix-assisted laser desorption/ionization (MALDI) for the mass spectrometric analysis of peptides and proteins had a dramatic impact on biological science. We now report that a wide variety of compounds, including peptides, proteins, and protein complexes, are transported directly from a solid-state small molecule matrix to gas-phase ions when placed into the vacuum of a mass spectrometer without the use of high voltage, a laser, or added heat. This ionization process produces ions having charge states similar to ESI, making the method applicable for high performance mass spectrometers designed for atmospheric pressure ionization. We demonstrate highly sensitive ionization using intermediate pressure MALDI and modified ESI sources. This matrix and vacuum assisted soft ionization method is suitable for the direct surface analysis of biological materials, including tissue, via mass spectrometry. PMID:23242551

  5. The galactic cosmic ray ionization rate

    PubMed Central

    Dalgarno, A.

    2006-01-01

    The chemistry that occurs in the interstellar medium in response to cosmic ray ionization is summarized, and a review of the ionization rates that have been derived from measurements of molecular abundances is presented. The successful detection of large abundances of H3+ in diffuse clouds and the recognition that dissociative recombination of H3+ is fast has led to an upward revision of the derived ionization rates. In dense clouds the molecular abundances are sensitive to the depletion of carbon monoxide, atomic oxygen, nitrogen, water, and metals and the presence of large molecules and grains. Measurements of the relative abundances of deuterated species provide information about the ion removal mechanisms, but uncertainties remain. The models, both of dense and diffuse clouds, that are used to interpret the observations may be seriously inadequate. Nevertheless, it appears that the ionization rates differ in dense and diffuse clouds and in the intercloud medium. PMID:16894166

  6. Ionization of NO at high temperature

    NASA Technical Reports Server (NTRS)

    Hansen, C. Frederick

    1991-01-01

    Space vehicles flying through the atmosphere at high speed are known to excite a complex set of chemical reactions in the atmospheric gases, ranging from simple vibrational excitation to dissociation, atom exchange, electronic excitation, ionization, and charge exchange. Simple arguments are developed for the temperature dependence of the reactions leading to ionization of NO, including the effect of vibrational electronic thermal nonequilibrium. NO ionization is the most important source of electrons at intermediate temperatures and at higher temperatures provides the trigger electrons that ionize atoms. Based on these arguments, recommendations are made for formulae which fit observed experimental results, and which include a dependence on both a heavy particle temperature and different vibration electron temperatures. In addition, these expressions will presumably provide the most reliable extrapolation of experimental results to much higher temperatures.

  7. Characterization of the CDMS Ionization Readout

    NASA Astrophysics Data System (ADS)

    Phipps, Arran

    2007-10-01

    Current cosmological models predict that a large portion of the total mass of the universe, about eighty percent, consists of putative dark matter. Theory predicts this dark matter may be in the form of particles constantly passing through the Earth. A class of these particles may interact with ordinary matter, earning the name weakly-interacting massive particles (WIMPs). The Cryogenic Dark Matter Search (CDMS) aims to directly detect the existence of WIMPs. CDMS has designed ZIP (Z-dependent Ionization & Phonon) detectors which measure phonon production and ionization of an interaction, making it possible to determine the interacting particle. The low-energy threshold of the ZIP detectors is determined by the signal-to-noise ratio of the ionization readout. A characterization of the signal-to-noise ratio of the ionization readout, along with possible modifications for improved sensitivity will be presented.

  8. The galactic cosmic ray ionization rate.

    PubMed

    Dalgarno, A

    2006-08-15

    The chemistry that occurs in the interstellar medium in response to cosmic ray ionization is summarized, and a review of the ionization rates that have been derived from measurements of molecular abundances is presented. The successful detection of large abundances of H(3)(+) in diffuse clouds and the recognition that dissociative recombination of H(3)(+) is fast has led to an upward revision of the derived ionization rates. In dense clouds the molecular abundances are sensitive to the depletion of carbon monoxide, atomic oxygen, nitrogen, water, and metals and the presence of large molecules and grains. Measurements of the relative abundances of deuterated species provide information about the ion removal mechanisms, but uncertainties remain. The models, both of dense and diffuse clouds, that are used to interpret the observations may be seriously inadequate. Nevertheless, it appears that the ionization rates differ in dense and diffuse clouds and in the intercloud medium.

  9. Chemi-ionization for Enhanced Plasma Densities

    NASA Astrophysics Data System (ADS)

    Ard, S.

    2016-12-01

    The Air Force has long considered ways of creating enhanced plasma density as a method of mitigating the detrimental effects of ionospheric density irregularities. Numerous easily photo-ionizable molecules have been released for study in this regard, yet this approach is inherently limited to daytime use. Recently attention has turned towards chemi-ionization. Several lanthanide metal oxides have bond strengths greater than their IP, such that M + O → MO+ + e- becomes energetically accessible. In 2013 the Metal Oxide Space Cloud (MOSC) mission released vaporized samarium in the lower ionosphere to study its potential as a chemi-ionization agent with atomic oxygen. While successful at producing enhanced densities, several results created questions about the underlying chemistry. This talk will focus on our lab's efforts supporting these releases, both in analysis of the principal thermochemistry and its effects on assessment of previous results, as well as ongoing experiments considering the potential of other chemi-ionization systems for future experiments.

  10. (Resonance ionization spectroscopy and its applications)

    SciTech Connect

    Ramsey, J.M.

    1990-10-11

    The Fifth International Symposium in Resonance Ionization Spectroscopy and Its Applications was attended. The Joint Research Centre of the European Communities at Ispra, Italy was also visited. The traveler presented an invited talk, chaired a meeting session and gave an impromptu presentation on how current laser technology limits the development of commercial instrumentation based upon Resonance Ionization Spectroscopy. The conference was truely international with scientists from 19 countries and less than 1/4 from the US. The meeting also provided a health mixture of experimentalists and theoreticians. Technical developments reported included the use of electric field ionization from laser prepared Rydberg states as a way to reduce background signals and commercial development of an optical parametric oscillator for replacing pulsed dye laser. A speaker from the Soviet Union suggested their willingness to market hardware they have developed based upon the resonance ionization technique.

  11. Fluctuations of induced charge in ionization detectors

    SciTech Connect

    Samedov, V. V.

    2016-12-15

    Fluctuations of charge induced by charge carriers on the detector electrodes make a significant contribution to the energy resolution of ionization detectors, namely, semiconductor detectors and gas and liquid ionization chambers. These fluctuations are determined by the capture of charge carriers, as they drift in the bulk of the detector under the action of an electric field, by traps. In this study, we give a correct mathematical description of charge induction on electrodes of an ionization detector for an arbitrary electric field distribution in the detector with consideration of charge carrier capture by traps. The characteristic function obtained in this study yields the general expression for the distribution function of the charge induced on the detector electrodes. The formulas obtained in this study are useful for analysis of the influence of charge carrier transport on energy resolution of ionization detectors.

  12. Which Stars Are Ionizing the Orion Nebula?

    NASA Astrophysics Data System (ADS)

    O’Dell, C. R.; Kollatschny, W.; Ferland, G. J.

    2017-03-01

    The common assumption that {θ }1 {Ori} {{C}} is the dominant ionizing source for the Orion Nebula is critically examined. This assumption underlies much of the existing analysis of the nebula. In this paper we establish through comparison of the relative strengths of emission lines with expectations from Cloudy models and through the direction of the bright edges of proplyds that {θ }2 {Ori} {{A}}, which lies beyond the Bright Bar, also plays an important role. {θ }1 {Ori} {{C}} does dominate ionization in the inner part of the Orion Nebula, but outside of the Bright Bar as far as the southeast boundary of the Extended Orion Nebula, {θ }2 {Ori} {{A}} is the dominant source. In addition to identifying the ionizing star in sample regions, we were able to locate those portions of the nebula in 3D. This analysis illustrates the power of MUSE spectral imaging observations to identify sources of ionization in extended regions.

  13. Ionization and positronium formation in noble gases

    SciTech Connect

    Marler, J.P.; Sullivan, J.P.; Surko, C.M.

    2005-02-01

    Absolute measurements are presented for the positron-impact cross sections for direct ionization and positronium formation of noble gas atoms in the range of energies from threshold to 90 eV. The experiment uses a cold, trap-based positron beam and the technique of studying positron scattering in a strong magnetic field. The current data show generally good, quantitative agreement with previous measurements taken using a qualitatively different method. However, significant differences in the cross sections for both direct ionization and positronium formation are also observed. An analysis is presented that yields another, independent measurement of the direct ionization and positronium formation cross sections that is in agreement with the present, direct measurements to within {+-}10% for argon, krypton, and xenon. Comparison with available theoretical predictions yields good quantitative agreement for direct ionization cross sections, and qualitative agreement in the case of positronium formation.

  14. Ionization energy of acetone by vacuum ultraviolet mass-analyzed threshold ionization spectrometry

    NASA Astrophysics Data System (ADS)

    Kim, Jae Han; Kang, Do Won; Hong, Yong Jun; Hwang, Hyonseok; Kim, Hong Lae; Kwon, Chan Ho

    2013-04-01

    Mass-analyzed threshold ionization (MATI) time-of-flight mass spectrometer using coherent vacuum ultraviolet (VUV) laser generated by four-wave difference frequency mixing (FWDFM) in Kr has been constructed and utilized to obtain the accurate ionization energy of acetone. From the MATI onsets measured from various applied pulsed fields, the ionization energy to the ionic ground state of acetone has been determined to be 9.7074 ± 0.0019 eV.

  15. Gas amplified ionization detector for gas chromatography

    DOEpatents

    Huston, Gregg C.

    1992-01-01

    A gas-amplified ionization detector for gas chromatrography which possesses increased sensitivity and a very fast response time. Solutes eluding from a gas chromatographic column are ionized by UV photoionization of matter eluting therefrom. The detector is capable of generating easily measured voltage signals by gas amplification/multiplication of electron products resulting from the UV photoionization of at least a portion of each solute passing through the detector.

  16. Diagnosing transient ionization in dynamic events

    NASA Astrophysics Data System (ADS)

    Doyle, J. G.; Giunta, A.; Madjarska, M. S.; Summers, H.; O'Mullane, M.; Singh, A.

    2013-09-01

    Aims: The present study aims to provide a diagnostic line ratio that will enable the observer to determine whether a plasma is in a state of transient ionization. Methods: We use the Atomic Data and Analysis Structure (ADAS) to calculate line contribution functions for two lines, Si iv 1394 Å and O iv 1401 Å, formed in the solar transition region. The generalized collisional-radiative theory is used. It includes all radiative and electron collisional processes, except for photon-induced processes. State-resolved direct ionization and recombination to and from the next ionization stage are also taken into account. Results: For dynamic bursts with a decay time of a few seconds, the Si iv 1394 Å line can be enhanced by a factor of 2-4 in the first fraction of a second with the peak in the line contribution function occurring initially at a higher electron temperature due to transient ionization compared to ionization equilibrium conditions. On the other hand, the O iv 1401 Å does not show such any enhancement. Thus the ratio of these two lines, which can be observed with the Interface Region Imaging Spectrograph, can be used as a diagnostic of transient ionization. Conclusions: We show that simultaneous high-cadence observations of two lines formed in the solar transition region may be used as a direct diagnostic of whether the observed plasma is in transient ionization. The ratio of these two lines can change by a factor of four in a few seconds owing to transient ionization alone.

  17. Field ionizing elements and applications thereof

    NASA Technical Reports Server (NTRS)

    Hartley, Frank T. (Inventor)

    2003-01-01

    A field ionizing element formed of a membrane that houses electrodes therein that are located closer to one another than the mean free path of the gas being ionized. The membrane includes a supporting portion, and a non supporting portion where the ions are formed. The membrane may be used as the front end for a number of different applications including a mass spectrometer, a thruster, an ion mobility element, or an electrochemical device such as a fuel cell.

  18. Tunneling ionization of vibrationally excited nitrogen molecules

    NASA Astrophysics Data System (ADS)

    Kornev, Aleksei S.; Zon, Boris A.

    2015-09-01

    Ionization of molecular nitrogen plays an important role in the process of light-filament formation in air. In the present paper we theoretically investigated tunneling ionization of the valence 3 σg and 1 πu shells in a N2 molecule using a strong near-infrared laser field. This research is based on our previously proposed theory of anti-Stokes-enhanced tunneling ionization with quantum accounting for the vibrationally excited states of the molecules [A. S. Kornev and B. A. Zon, Phys. Rev. A 86, 043401 (2012), 10.1103/PhysRevA.86.043401]. We demonstrated that if the N2 molecule is ionized from the ground vibrational state, then the contribution of the 1 πu orbital is 0.5%. In contrast, for vibrationally excited states with a certain angle between the light polarization vector and the molecule axis, both shells can compete and even reverse their contributions due to the anti-Stokes mechanism. The structure constants of molecular orbitals are extracted from numerical solutions to the Hartree-Fock equations. This approach correctly takes into account the exchange interaction. Quantum consideration of vibrational motion results in the occurrence of the critical vibrational state, the tunneling ionization from which has the maximum rate. The numbers of the critical vibrational states are different for different valence shells. In addition, quantum description of vibrations changes the rate of ionization from the ground vibrational state by 20%-40% in comparison with the quasiclassical results.

  19. Neutral depletion versus repletion due to ionization

    SciTech Connect

    Fruchtman, A.; Makrinich, G.; Raimbault, J.-L.; Liard, L.; Rax, J.-M.; Chabert, P.

    2008-05-15

    Recent theoretical analyses which predicted unexpected effects of neutral depletion in both collisional and collisionless plasmas are reviewed. We focus on the depletion of collisionless neutrals induced by strong ionization of a collisionless plasma and contrast this depletion with the effect of strong ionization on thermalized neutrals. The collisionless plasma is analyzed employing a kinetic description. The collisionless neutrals and the plasma are coupled through volume ionization and wall recombination only. The profiles of density and pressure both of the plasma and of the neutral-gas and the profile of the ionization rate are calculated. It is shown that for collisionless neutrals the ionization results in neutral depletion, while when neutrals are thermalized the ionization induces a maximal neutral-density at the discharge center, which we call neutral repletion. The difference between the two cases stems from the relation between the neutral density and pressure. The pressure of the collisionless neutral-gas turns out to be maximal where its density is minimal, in contrast to the case of a thermalized neutral gas.

  20. Resonant effects in above-threshold ionization

    NASA Astrophysics Data System (ADS)

    Hertlein, Marcus P.

    2000-09-01

    The ionization of noble gases in high intensity laser fields produces an electron spectrum with characteristic peaks corresponding to atomic levels of the atom. While many of the features in the low energy part of the spectrum have been explained qualitatively, current models are incomplete and are not able to account for the recurrence of ionization probability for higher energy electrons. In particular, one of the basic questions arising is the importance of multiple ionization in these spectra. While the light intensities are in the regime where multiple ionization is known to occur, it was not clear whether the higher energy (or plateau) electrons are a result of this, and whether multiple ionization even leaves a signature in the electron spectrum. In this dissertation, we use several experimental techniques to explore this problem in argon. Our results show that although multiple ionization occurs, electrons from this process do not appear in the observed electron spectrum. Furthermore, the appearance intensities of the peaks visible in the plateau region of the electron spectrum and of the resonance peaks in the well- understood low energy part show a strong correlation, suggestion a common origin of production. Accurate computer simulations of the process, using a single- active-electron model, reproduce all essential features of the experimental spectra. Our results support the conclusion that all high energy electrons observed in our experiments can be explained with single-electron effects.

  1. Multiple ionization of argon by helium ions

    NASA Astrophysics Data System (ADS)

    Montanari, C. C.; Miraglia, J. E.

    2016-09-01

    We apply the continuum distorted-wave eikonal initial state and the independent electron model to describe the multiple ionization of Ar by He2+ and He+ in the energy range 0.1-10 Mev amu-1. Auger-like post collisional processes are included, which enhance the high energy multiple ionization cross sections via ionization of the inner shells. All Ar electrons (K, L and M-shells) have been included in these calculations. The results agree well with the experimental data at high energies, where the post-collisional ionization is the main contribution. At intermediate impact energies the description is also good though it tends to overestimate the triple and quadruple ionization data at intermediate energies. We analyze this by comparing the present results for He+2 in Ar, with previous ones for He+2 in Ne and Kr. It was found that the theoretical description improves from Ne to Ar and Kr, with the latter being nicely described even at intermediate energies. The present formalism is also tested for Ar inner shell and total ionization cross sections. In all the cases the results above 0.1 MeV amu-1 are quite reasonable, as compared with the experimental data available and with the ECPSSR values.

  2. The oncogenic action of ionizing radiation on rat skin

    SciTech Connect

    Burns, F.J.

    1991-01-01

    Progress has occurred in several areas corresponding to the specific aims of the proposal: (1) Progression and multiple events in radiation carcinogenesis of rat skin as a function of LET; (2) cell cycle kinetics of irradiated rat epidermis as determined by double labeling and double emulsion autoradiography; (3) oncogene activation detected by in situ hybridization in radiation-induced rat skin tumors; (4) amplification of the c-myc oncogene in radiation-induced rat skin tumors as a function of LET; and (5) transformation of rat skin keratinocytes by ionizing radiation in combination with c-Ki-ras and c-myc oncogenes. 111 refs., 13 figs., 12 tabs.

  3. Caustics and catastrophes in above-threshold ionization

    NASA Astrophysics Data System (ADS)

    Kelvich, S. A.; Becker, W.; Goreslavski, S. P.

    2017-08-01

    Low-energy above-threshold ionization by a midinfrared laser field is investigated in terms of a commonly used semiclassical model. The mapping of the initial conditions (initial transverse velocity and initial phase of the field) on the final drift momenta that is mediated by Newton's equation of motion is approximated by three Coulomb interactions, which occur at the exit of the tunnel and during the subsequent hard and soft interactions that occur when the electron revisits the ion. The mapping exhibits a particular caustic structure in the area of the low-energy structure, which has the shape of the butterfly catastrophe.

  4. Nrf2 promotes survival following exposure to ionizing radiation.

    PubMed

    Sekhar, Konjeti R; Freeman, Michael L

    2015-11-01

    Nrf2 is a transcription factor that promotes antioxidant and drug-metabolizing gene expression. It also regulates the transcription of genes involved in carbohydrate and lipid metabolism, NADPH regeneration, and heme and iron metabolism, as well as proteasome metabolism. Emerging research has identified Nrf2 as a critical factor for promoting survival of mammalian cells subjected to ionizing radiation. At a mechanistic level, Nrf2 promotes the repair of DNA damage and drives detoxification of superoxide that is generated hours to days after irradiation. This review summarizes research in these areas and discusses targeting of Nrf2 in radiation-resistant cancer and Nrf2׳s role in mitigating acute radiation syndrome.

  5. About AGN ionization echoes, thermal echoes and ionization deficits in low-redshift Lyα blobs

    NASA Astrophysics Data System (ADS)

    Schirmer, Mischa; Malhotra, Sangeeta; Levenson, Nancy A.; Fu, Hai; Davies, Rebecca L.; Keel, William C.; Torrey, Paul; Bennert, Vardha N.; Pancoast, Anna; Turner, James E. H.

    2016-12-01

    We report the discovery of 14 Lyα blobs (LABs) at z ˜ 0.3, existing at least 4-7 billion years later in the Universe than all other LABs known. Their optical diameters are 20-70 kpc, and GALEX data imply Lyα luminosities of (0.4-6.3) × 1043 erg s-1. Contrary to high-z LABs, they live in low-density areas. They are ionized by AGN, suggesting that cold accretion streams as a power source must deplete between z = 2 and 0.3. We also show that transient AGN naturally explain the ionization deficits observed in many LABs. Their Lyα and X-ray fluxes decorrelate below ≲106 years because of the delayed escape of resonantly scattering Lyα photons. High Lyα luminosities do not require currently powerful AGN, independent of obscuration. Chandra X-ray data reveal intrinsically weak AGN, confirming the luminous optical nebulae as impressive ionization echoes. For the first time, we also report mid-infrared thermal echoes from the dusty tori. We conclude that the AGN have faded by three to four orders of magnitude within the last 104-5 years, leaving fossil UV, optical and thermal radiation behind. The host galaxies belong to the group of previously discovered Green Bean galaxies (GBs). Gemini optical imaging reveals smooth spheres, mergers, spectacular outflows and ionization cones. Because of their proximity and high flux densities, GBs are perfect targets to study AGN feedback, mode switching and the Lyα escape. The fully calibrated, co-added optical FITS images are publicly available.

  6. Helium Ionization in the Diffuse Ionized Gas Surrounding UCH ii Regions

    NASA Astrophysics Data System (ADS)

    Anish Roshi, D.; Churchwell, E.; Anderson, L. D.

    2017-04-01

    We present measurements of the singly ionized helium-to-hydrogen ratio ({n}{{He}+}/{n}{{{H}}+}) toward diffuse gas surrounding three ultracompact H ii (UCH ii) regions: G10.15-0.34, G23.46-0.20, and G29.96-0.02. We observe radio recombination lines of hydrogen and helium near 5 GHz using the GBT to measure the {n}{{He}+}/{n}{{{H}}+} ratio. The measurements are motivated by the low helium ionization observed in the warm ionized medium and in the inner Galaxy diffuse ionized regions. Our data indicate that the helium is not uniformly ionized in the three observed sources. Helium lines are not detected toward a few observed positions in sources G10.15-0.34 and G23.46-0.20, and the upper limits of the {n}{{He}+}/{n}{{{H}}+} ratio obtained are 0.03 and 0.05, respectively. The selected sources harbor stars of type O6 or hotter as indicated by helium line detection toward the bright radio continuum emission from the sources with mean {n}{{He}+}/{n}{{{H}}+} value 0.06 ± 0.02. Our data thus show that helium in diffuse gas located a few parsecs away from the young massive stars embedded in the observed regions is not fully ionized. We investigate the origin of the nonuniform helium ionization and rule out the possibilities (a) that the helium is doubly ionized in the observed regions and (b) that the low {n}{{He}+}/{n}{{{H}}+} values are due to additional hydrogen ionizing radiation produced by accreting low-mass stars. We find that selective absorption of ionizing photons by dust can result in low helium ionization but needs further investigation to develop a self-consistent model for dust in H ii regions.

  7. Helium Ionization in the Diffuse Ionized Gas Surrounding UCH ii Regions

    NASA Astrophysics Data System (ADS)

    Roshi, D. Anish; Churchwell, E.; Anderson, L. D.

    2017-04-01

    We present measurements of the singly ionized helium-to-hydrogen ratio ({n}{{He}+}/{n}{{{H}}+}) toward diffuse gas surrounding three ultracompact H ii (UCH ii) regions: G10.15-0.34, G23.46-0.20, and G29.96-0.02. We observe radio recombination lines of hydrogen and helium near 5 GHz using the GBT to measure the {n}{{He}+}/{n}{{{H}}+} ratio. The measurements are motivated by the low helium ionization observed in the warm ionized medium and in the inner Galaxy diffuse ionized regions. Our data indicate that the helium is not uniformly ionized in the three observed sources. Helium lines are not detected toward a few observed positions in sources G10.15-0.34 and G23.46-0.20, and the upper limits of the {n}{{He}+}/{n}{{{H}}+} ratio obtained are 0.03 and 0.05, respectively. The selected sources harbor stars of type O6 or hotter as indicated by helium line detection toward the bright radio continuum emission from the sources with mean {n}{{He}+}/{n}{{{H}}+} value 0.06 ± 0.02. Our data thus show that helium in diffuse gas located a few parsecs away from the young massive stars embedded in the observed regions is not fully ionized. We investigate the origin of the nonuniform helium ionization and rule out the possibilities (a) that the helium is doubly ionized in the observed regions and (b) that the low {n}{{He}+}/{n}{{{H}}+} values are due to additional hydrogen ionizing radiation produced by accreting low-mass stars. We find that selective absorption of ionizing photons by dust can result in low helium ionization but needs further investigation to develop a self-consistent model for dust in H ii regions.

  8. IONIZATION IN ATMOSPHERES OF BROWN DWARFS AND EXTRASOLAR PLANETS. V. ALFVÉN IONIZATION

    SciTech Connect

    Stark, C. R.; Helling, Ch.; Rimmer, P. B.; Diver, D. A.

    2013-10-10

    Observations of continuous radio and sporadic X-ray emission from low-mass objects suggest they harbor localized plasmas in their atmospheric environments. For low-mass objects, the degree of thermal ionization is insufficient to qualify the ionized component as a plasma, posing the question: what ionization processes can efficiently produce the required plasma that is the source of the radiation? We propose Alfvén ionization as a mechanism for producing localized pockets of ionized gas in the atmosphere, having sufficient degrees of ionization (≥10{sup –7}) that they constitute plasmas. We outline the criteria required for Alfvén ionization and demonstrate its applicability in the atmospheres of low-mass objects such as giant gas planets, brown dwarfs, and M dwarfs with both solar and sub-solar metallicities. We find that Alfvén ionization is most efficient at mid to low atmospheric pressures where a seed plasma is easier to magnetize and the pressure gradients needed to drive the required neutral flows are the smallest. For the model atmospheres considered, our results show that degrees of ionization of 10{sup –6}-1 can be obtained as a result of Alfvén ionization. Observable consequences include continuum bremsstrahlung emission, superimposed with spectral lines from the plasma ion species (e.g., He, Mg, H{sub 2}, or CO lines). Forbidden lines are also expected from the metastable population. The presence of an atmospheric plasma opens the door to a multitude of plasma and chemical processes not yet considered in current atmospheric models. The occurrence of Alfvén ionization may also be applicable to other astrophysical environments such as protoplanetary disks.

  9. Photo-ionization rate coefficients for the rare gases

    NASA Astrophysics Data System (ADS)

    Pang, Xuexia

    2005-01-01

    By introducing the converting method from electron-impact ionization cross sections to rate coefficients through using a semi-experiential formula, we try to probe a semi-experiential formula for converting the photo-ionization cross sections into photo-ionization rate coefficient. It"s found that photo-ionization rate coefficient is direct proportion to photo-ionization cross sections, the rate S is related with light resource.

  10. Adverse cutaneous effects of ionizing and non-ionizing electromagnetic radiation.

    PubMed

    Testa, E R; Cooper, J S

    1980-03-01

    Modern man is constantly exposed to many forms of electromagnetic radiation, both ionizing and non-ionizing. Although many uses of electromagnetic radiation artfully administered serve man well, injudicious exposure carries a potential for harm. Various types of electromagnetic radiation and possible hazards from them are discussed.

  11. Simultaneous resonant enhanced multiphoton ionization and electron avalanche ionization in gas mixtures

    SciTech Connect

    Shneider, Mikhail N.; Zhang Zhili; Miles, Richard B.

    2008-07-15

    Resonant enhanced multiphoton ionization (REMPI) and electron avalanche ionization (EAI) are measured simultaneously in Ar:Xe mixtures at different partial pressures of mixture components. A simple theory for combined REMPI+EAI in gas mixture is developed. It is shown that the REMPI electrons seed the avalanche process, and thus the avalanche process amplifies the REMPI signal. Possible applications are discussed.

  12. The ionizing star of the North America and Pelican nebulae

    NASA Astrophysics Data System (ADS)

    Comerón, F.; Pasquali, A.

    2005-02-01

    We present the results of a search for the ionizing star of the North America (NGC 7000) and the Pelican (IC 5070) nebulae complex. The application of adequate selection criteria to the 2MASS JH KS broad-band photometry allows us to narrow the search down to 19 preliminary candidates in a circle of 0o 5 radius containing most of the L935 dark cloud that separates both nebulae. Follow-up near-infrared spectroscopy shows that most of these objects are carbon stars and mid-to-late-type giants, including some AGB stars. Two of the three remaining objects turn out to be later than spectral type B and thus cannot account for the ionization of the nebula, but a third object, 2MASS J205551.25+435224.6, has infrared properties consistent with it being a mid O-type star at the distance of the nebulae complex and reddened by AV ≃ 9.6. We confirm its O5V spectral type by means of visible spectroscopy in the blue. This star has the spectral type required by the ionization conditions of the nebulae and photometric properties consistent with the most recent estimates of their distance. Moreover, it lies close to the geometric center of the complex that other studies have proposed as the most likely location for the ionizing star, and is also very close to the position inferred from the morphology of cloud rims detected in radio continuum. Given the fulfillment of all the conditions and the existence of only one star in the whole search area that satisfies them, we thus propose 2MASS J205551.25+435224.6 as the ionizing star of the North America/Pelican complex. Based on observations collected at the Centro Astronómico Hispano-Alemán (CAHA) at Calar Alto, operated jointly by the Max-Planck Institut für Astronomie and the Instituto de Astrofísica de Andalucía (CSIC). Figure 1 is only available in electronic form at http://www.edpsciences.org

  13. Apparatus and method for selective area deposition of thin films on electrically biased substrates

    DOEpatents

    Zuhr, Raymond A.; Haynes, Tony E.; Golanski, Andrzej

    1994-01-01

    An ion beam deposition process for selective area deposition on a polarized substrate uses a potential applied to the substrate which allows the ionized particles to reach into selected areas for film deposition. Areas of the substrate to be left uncoated are held at a potential that repells the ionized particles.

  14. Apparatus and method for selective area deposition of thin films on electrically biased substrates

    DOEpatents

    Zuhr, Raymond A.; Haynes, Tony E.; Golanski, Andrzej

    1999-01-01

    An ion beam deposition process for selective area deposition on a polarized substrate uses a potential applied to the substrate which allows the ionized particles to reach into selected areas for film deposition. Areas of the substrate to be left uncoated are held at a potential that repells the ionized particles.

  15. Apparatus and method for selective area deposition of thin films on electrically biased substrates

    DOEpatents

    Zuhr, R.A.; Haynes, T.E.; Golanski, A.

    1999-06-08

    An ion beam deposition process for selective area deposition on a polarized substrate uses a potential applied to the substrate which allows the ionized particles to reach into selected areas for film deposition. Areas of the substrate to be left uncoated are held at a potential that repels the ionized particles. 3 figs.

  16. Dispersal of molecular clouds by ionizing radiation

    NASA Astrophysics Data System (ADS)

    Walch, S. K.; Whitworth, A. P.; Bisbas, T.; Wünsch, R.; Hubber, D.

    2012-11-01

    Feedback from massive stars is believed to be a key element in the evolution of molecular clouds. We use high-resolution 3D smoothed particle hydrodynamics simulations to explore the dynamical effects of a single O7 star-emitting ionizing photons at 1049 s-1 and located at the centre of a molecular cloud with mass 104 M⊙ and radius 6.4 pc; we also perform comparison simulations in which the ionizing star is removed. The initial internal structure of the cloud is characterized by its fractal dimension, which we vary between D=2.0 and 2.8, and the standard deviation of the approximately log-normal initial densityPDF, which is σ10 = 0.38 for all clouds. (i) As regards star formation, in the short term ionizing feedback is positive, in the sense that star formation occurs much more quickly (than in the comparison simulations), in gas that is compressed by the high pressure of the ionized gas. However, in the long term ionizing feedback is negative, in the sense that most of the cloud is dispersed with an outflow rate of up to ˜10-2 M⊙yr-1, on a time-scale comparable with the sound-crossing time for the ionized gas (˜1-2 Myr ), and triggered star formation is therefore limited to a few per cent of the cloud's mass. We will describe in greater detail the statistics of the triggered star formation in a companion paper. (ii) As regards the morphology of the ionization fronts (IFs) bounding the H II region and the systematics of outflowing gas, we distinguish two regimes. For low D≲2.2, the initial cloud is dominated by large-scale structures, so the neutral gas tends to be swept up into a few extended coherent shells, and the ionized gas blows out through a few large holes between these shells; we term these H II regions shell dominated. Conversely, for high D≳2.6, the initial cloud is dominated by small-scale structures, and these are quickly overrun by the advancing IF, thereby producing neutral pillars protruding into the H II region, whilst the ionized gas

  17. Resonant ionization spectroscopy of autoionizing Rydberg states in cobalt and redetermination of its ionization potential

    DOE PAGES

    Liu, Yuan; Gottwald, T.; Mattolat, C.; ...

    2017-03-20

    We obtained multi-step resonance ionization spectroscopy of cobalt using a hot-cavity laser ion source and three Ti:Sapphire lasers. Furthermore, the photoionization spectra revealed members of five new autoionizing Rydberg series that originate from three different lower levels of 3d74s5s h4F9/2, 3d74s4d f4G11/2, and 3d74s4d f4H13/2 and converge to the first four excited states of singly ionized Co. Our analyses of the Rydberg series yield 63564.689 0.036 cm-1 as the first ionization potential of Co, which is an order of magnitude more accurate than the previous estimation. Using a three-step resonance ionization scheme that employs an autoinizing Rydberg state in themore » last transition, we obtained an overall ionization efficiency of about 18% for Co.« less

  18. Ionization Time and Exit Momentum in Strong-Field Tunnel Ionization.

    PubMed

    Teeny, Nicolas; Yakaboylu, Enderalp; Bauke, Heiko; Keitel, Christoph H

    2016-02-12

    Tunnel ionization belongs to the fundamental processes of atomic physics. The so-called two-step model, which describes the ionization as instantaneous tunneling at the electric field maximum and classical motion afterwards with zero exit momentum, is commonly employed to describe tunnel ionization in adiabatic regimes. In this contribution, we show by solving numerically the time-dependent Schrödinger equation in one dimension and employing a virtual detector at the tunnel exit that there is a nonvanishing positive time delay between the electric field maximum and the instant of ionization. Moreover, we find a nonzero exit momentum in the direction of the electric field. To extract proper tunneling times from asymptotic momentum distributions of ionized electrons, it is essential to incorporate the electron's initial momentum in the direction of the external electric field.

  19. Management of ionizing radiation injuries and illnesses, Part 3: Radiobiology and health effects of ionizing radiation.

    PubMed

    Christensen, Doran M; Livingston, Gordon K; Sugarman, Stephen L; Parillo, Steven J; Glassman, Erik S

    2014-07-01

    Ionizing radiation exposure can induce profound changes in intracellular components, potentially leading to diverse health effects in exposed individuals. Any cellular component can be damaged by radiation, but some components affect cellular viability more profoundly than others. The ionization caused by radiation lasts longer than the initial inciting incident, continuing as 1 ionization incident causes another. In some cases, damage to DNA can lead to cellular death at mitosis. In other cases, activation of the genetic machinery can lead to a genetic cascade potentially leading to mutations or cell death by apoptosis. In the third of 5 articles on the management of injuries and illnesses caused by ionizing radiation, the authors provide a clinically relevant overview of the pathophysiologic process associated with potential exposure to ionizing radiation.

  20. Resonant ionization spectroscopy of autoionizing Rydberg states in cobalt and redetermination of its ionization potential

    NASA Astrophysics Data System (ADS)

    Liu, Y.; Gottwald, T.; Mattolat, C.; Wendt, K.

    2017-04-01

    Multi-step resonance ionization spectroscopy of cobalt has been performed using a hot-cavity laser ion source and three Ti:Sapphire lasers. The photoionization spectra revealed members of five new autoionizing Rydberg series that originate from three different lower levels of 3d 74s5s h 4F9/2, 3d 74s4d f 4G11/2, and 3d 74s4d f 4H13/2 and converge to the first four excited states of singly ionized Co. The analyses of the Rydberg series yield 63 564.689 ± 0.036 cm‑1 as the first ionization potential of Co, which is an order of magnitude more accurate than the previous estimation. Using a three-step resonance ionization scheme that employs an autoinizing Rydberg state in the last transition, we obtained an overall ionization efficiency of about 18% for Co. ).

  1. Laboratory simulation of cometary neutral gas ionization

    NASA Technical Reports Server (NTRS)

    Chang, Tsuey-Fen; Rahman, H. U.; White, R. S.

    1989-01-01

    The laboratory simulation of the interaction of the solar wind with a comet is used to study the cometary neural gas ionization. The experiment is carried out in the UCR T-1 facility with an ice ball as the comet model. Photographs and data are taken with a variety of values of the solar wind velocity, interplanetary magnetic field (IMF), and comet configurations. The results show that the cometary neutral gas ionization depends on both the velocity of the solar wind and the interplanetary magnetic field. The plasma cloud surrounding the comet is visible only when the solar wind velocity and IMF are both above certain minimum values. This velocity dependent phenomena is explained by Alfven's critical ionization velocity effect. The critical magnetic field may be explained by assuming two stream lower hybrid instability as a triggering mechanism for the ionization of the neutral gas by plasma flow. Critical upper and lower limits for the magnetic field, required by anomalous ionization, are also derived that satisfy the experimental observations.

  2. Meteoric Ionization Layers in the Martian Atmosphere

    NASA Astrophysics Data System (ADS)

    Pesnell, W. D.; Grebowsky, J. M.

    1997-12-01

    Mars, like the other planets, is bombarded by meteorites. At least two families of particles impact the planets: sporadic and shower. In the terrestrial atmosphere both families cause sporadic-E layers when the introduced material is ionized by charge-exchange, photoionization, or impact ionization. Narrow layers of ionized material are produced when the long-lived metallic ions are compressed by tidal or gravity wave motions in the atmosphere. We will examine how the ion-neutral chemistry and dynamics of the Martian atmosphere affect the deposited meteoric material. Our emphasis is on magnesium, an easily ionized species that is a major component of the meteoric debris. The parameters that affect the meteoric ionization differ between Earth and Mars. In particular, the atmospheric compositions and ionospheric densities differ. Further, the lower atmospheric pressure on Mars means lower altitudes for the bulk of the atmospheric ablation of the meteorites. However, the range of atmospheric density variation at high altitudes is greater at Mars than at Earth, so that sputtering of high speed shower streams which occurs at high altitudes may be relatively more important at Mars than Earth.

  3. Low latitude middle atmosphere ionization studies

    NASA Technical Reports Server (NTRS)

    Bassi, J. P.

    1976-01-01

    Low latitude middle atmosphere ionization was studied with data obtained from three blunt conductivity probes and one Gerdien condenser. An investigation was conducted into the effects of various ionization sources in the 40 to 65 Km altitude range. An observed enhancement of positive ion conductivity taking place during the night can be explained by an atmsopheric effect, with cosmic rays being the only source of ionization only if the ion-ion recombination coefficient (alpha sub i) is small(10 to the -7 power cu cm/s) and varies greatly with altitude. More generally accepted values of alpha sub i ( approximately equal to 3x10 to the -7 power cu cm/s) require an additional source of ionization peaking at about 65 Km, and corresponding approximately to the integrated effect of an X-ray flux measured on a rocket flown in conjunction with the ionization measurements. The reasonable assumption of an alpha sub i which does not vary with altitude in the 50-70 Km range implies an even greater value alpha sub i and a more intense and harder X-ray spectrum.

  4. Conceptual basis of resonance ionization spectroscopy

    SciTech Connect

    Payne, M.G.

    1984-04-01

    Resonance Ionization Spectroscopy (RIS) can b defined as a state-selective detection process in which tunable lasers are used to promote transitions from the selected state of the atoms or molecules in question to higher states, one of which will be ionized by the absorption of another photon. At least one resonance step is used in the stepwise ionization process, and it has been shown that the ionization probability of the spectroscopically selected species can nearly always be made close to unity. Since measurements of the number of photoelectrons or ions can be made very precisely and even one electron (or under vacuum conditions, one ion) can be detected, the technique can be used to make quantitative measurements of very small populations of the state-selected species. Counting of individual atoms has special meaning for detection of rare events. The ability to make saturated RIS measurements opens up a wide variety of applications to both basic and applied research. We view RIS as a specific type of multi-photon ionization in which the goal is to make quantitative measurements of quantum-selected populations in atomic or molecular systems. 16 references.

  5. Organic materials and devices for detecting ionizing radiation

    DOEpatents

    Doty, F. Patrick; Chinn, Douglas A.

    2007-03-06

    A .pi.-conjugated organic material for detecting ionizing radiation, and particularly for detecting low energy fission neutrons. The .pi.-conjugated materials comprise a class of organic materials whose members are intrinsic semiconducting materials. Included in this class are .pi.-conjugated polymers, polyaromatic hydrocarbon molecules, and quinolates. Because of their high resistivities (.gtoreq.10.sup.9 ohmcm), these .pi.-conjugated organic materials exhibit very low leakage currents. A device for detecting and measuring ionizing radiation can be made by applying an electric field to a layer of the .pi.-conjugated polymer material to measure electron/hole pair formation. A layer of the .pi.-conjugated polymer material can be made by conventional polymer fabrication methods and can be cast into sheets capable of covering large areas. These sheets of polymer radiation detector material can be deposited between flexible electrodes and rolled up to form a radiation detector occupying a small volume but having a large surface area. The semiconducting polymer material can be easily fabricated in layers about 10 .mu.m to 100 .mu.m thick. These thin polymer layers and their associated electrodes can be stacked to form unique multi-layer detector arrangements that occupy small volume.

  6. Ionized gas clouds near the Sagittarius Arm tangent

    NASA Astrophysics Data System (ADS)

    Hou, Li-Gang; Dong, Jian; Gao, Xu-Yang; Han, Jin-Lin

    2017-04-01

    Radio recombination lines (RRLs) are the best tracers of ionized gas. Simultaneous observations of multi-transitions of RRLs can significantly improve survey sensitivity. We conducted pilot RRL observations near the Sagittarius Arm tangent by using the 65-m Shanghai Tian Ma Radio Telescope (TMRT) equipped with broadband feeds and a digital backend. Six hydrogen RRLs (H96 α - H101α) at C band (6289 MHz-7319 MHz) were observed simultaneously toward a sky area of 2° × 1.2° by using on-the-fly mapping mode. These transitions were then stacked together for detection of ionized gas. Star forming complexes G48.6+0.1 and G49.5-0.3 were detected in the integrated intensity map. We found agreements between our measured centroid velocities and previous results for the 21 known HII regions in the mapped area. For more than 80 cataloged HII region candidates without previous RRL measurements, we obtained new RRL spectra at 30 targeted positions. In addition, we detected 25 new discrete RRL sources with spectral S/N > 5 σ, and they were not listed in the catalogs of previously known HII regions. The distances for 44 out of these 55 new RRL sources were estimated.

  7. Laser induced avalanche ionization in gases or gas mixtures with resonantly enhanced multiphoton ionization or femtosecond laser pulse pre-ionization

    SciTech Connect

    Shneider, Mikhail N.; Miles, Richard B.

    2012-08-15

    The paper discusses the requirements for avalanche ionization in gas or gas mixtures initiated by REMPI or femtosecond-laser pre-ionization. Numerical examples of dependencies on partial composition for Ar:Xe gas mixture with REMPI of argon and subsequent classic avalanche ionization of Xe are presented.

  8. Photoelectron circular dichroism in different ionization regimes

    NASA Astrophysics Data System (ADS)

    Wollenhaupt, Matthias

    2016-12-01

    Photoelectron circular dichroism (PECD) describes an asymmetry in the photoelectron angular distribution (PAD) from photoionization of randomly oriented enantiomers with circularly polarized light. Beaulieu et al present a comprehensive set of measured PADs from multiphoton ionization of limonene and fenchone in different ionization regimes (multiphoton and tunneling) and analyze the resulting PECD (Beaulieu et al 2016 New J. Phys. 18 102002). From their observations the authors conclude that the PECD is universal in the sense that the molecular chirality is encoded in the PAD independent of the ionization regime. The analysis is supplemented by a classical model based on electron scattering in a chiral potential. The paper presents beautiful data and is an important step towards a more complete physical picture of PECD. The results and their interpretation stimulate the ongoing vivid debate on the role of resonances in multiphoton PECD.

  9. Pediatric Exposures to Ionizing Radiation: Carcinogenic Considerations

    PubMed Central

    Kutanzi, Kristy R.; Lumen, Annie; Koturbash, Igor; Miousse, Isabelle R.

    2016-01-01

    Children are at a greater risk than adults of developing cancer after being exposed to ionizing radiation. Because of their developing bodies and long life expectancy post-exposure, children require specific attention in the aftermath of nuclear accidents and when radiation is used for diagnosis or treatment purposes. In this review, we discuss the carcinogenic potential of pediatric exposures to ionizing radiation from accidental, diagnostic, and therapeutic modalities. Particular emphasis is given to leukemia and thyroid cancers as consequences of accidental exposures. We further discuss the evidence of cancers that arise as a result of radiotherapy and conclude the review with a summary on the available literature on the links between computer tomography (CT) and carcinogenesis. Appropriate actions taken to mitigate or minimize the negative health effects of pediatric exposures to ionizing radiation and future considerations are discussed. PMID:27801855

  10. Theoretical IR spectra of ionized naphthalene

    NASA Technical Reports Server (NTRS)

    Pauzat, F.; Talbi, D.; Miller, M. D.; DeFrees, D. J.; Ellinger, Y.

    1992-01-01

    We report the results of a theoretical study of the effect of ionization on the IR spectrum of naphthalene, using ab initio molecular orbital theory. For that purpose we determined the structures, band frequencies, and intensities of neutral and positively ionized naphthalene. The calculated frequencies and intensities allowed an assignment of the most important bands appearing in the newly reported experimental spectrum of the positive ion. Agreement with the experimental spectrum is satisfactory enough to take into consideration the unexpected and important result that ionization significantly affects the intensities of most vibrations. A possible consequence on the interpretation of the IR interstellar emission, generally supposed to originate from polycyclic aromatic hydrocarbons (PAHs), is briefly presented.

  11. Ionization-chamber smoke detector system

    DOEpatents

    Roe, Robert F.

    1976-10-19

    This invention relates to an improved smoke-detection system of the ionization-chamber type. In the preferred embodiment, the system utilizes a conventional detector head comprising a measuring ionization chamber, a reference ionization chamber, and a normally non-conductive gas triode for discharging when a threshold concentration of airborne particulates is present in the measuring chamber. The improved system is designed to reduce false alarms caused by fluctuations in ambient temperature. Means are provided for periodically firing the gas discharge triode and each time recording the triggering voltage required. A computer compares each triggering voltage with its predecessor. The computer is programmed to energize an alarm if the difference between the two compared voltages is a relatively large value indicative of particulates in the measuring chamber and to disregard smaller differences typically resulting from changes in ambient temperature.

  12. Capillary electrophoresis electrospray ionization mass spectrometry interface

    DOEpatents

    Smith, Richard D.; Severs, Joanne C.

    1999-01-01

    The present invention is an interface between a capillary electrophoresis separation capillary end and an electrospray ionization mass spectrometry emitter capillary end, for transporting an anolyte sample from a capillary electrophoresis separation capillary to a electrospray ionization mass spectrometry emitter capillary. The interface of the present invention has: (a) a charge transfer fitting enclosing both of the capillary electrophoresis capillary end and the electrospray ionization mass spectrometry emitter capillary end; (b) a reservoir containing an electrolyte surrounding the charge transfer fitting; and (c) an electrode immersed into the electrolyte, the electrode closing a capillary electrophoresis circuit and providing charge transfer across the charge transfer fitting while avoiding substantial bulk fluid transfer across the charge transfer fitting. Advantages of the present invention have been demonstrated as effective in providing high sensitivity and efficient analyses.

  13. Dynamics of cluster dissociation following multiphoton ionization

    SciTech Connect

    Castleman, A.W.

    1986-01-01

    A major advance in the study of unimolecular dissociation and the spectroscopy of clusters has become available through the use of multiphoton ionization coupled with a reflectron introduced into the drift region of a time-of-flight mass spectrometer. Using single and two-color tunable pulsed lasers, the excess energy introduced into a cluster can be well controlled. The power of this method is demonstrated by the results of recent investigations of hydrogen-bonded clusters which, following ionization, lead to an internal ion-molecule reaction, and cluster fragmentation. The role of dissociation and the influence of the thermochemical stability of cluster ions in effecting the appearance of magic numbers in certain cluster distributions is discussed. The application of this method in determining ionization potentials of probe molecules following successive clustering with a solvent species is also presented.

  14. Theoretical determinations of ionization potentials of dopamine

    NASA Astrophysics Data System (ADS)

    Lu, J. F.; Yu, Z. Y.

    2013-04-01

    Adiabatic and vertical ionization potentials (IPs) of nine conformers of dopamine in the gas phase are determined using density functional theory (DFT) B3LYP, B3P86, B3PW91 methods and high level ab initio HF method with 6-311++G** basis set, respectively. And the nine stable cationic states have been found in the ionization process of dopamine. Vertical ionization potentials of nine conformers of dopamine are calculated using the older outer-valence Green's function (OVGF) calculations at 6-311++G** basis set. Vibrational frequencies and infrared spectrum intensities of G1b and G1b+ at B3LYP/6-311++G** level are discussed.

  15. Vibrationally assisted below-threshold ionization

    NASA Astrophysics Data System (ADS)

    Horton, Spencer L.; Liu, Yusong; Chakraborty, Pratip; Matsika, Spiridoula; Weinacht, Thomas

    2017-06-01

    We perform time-resolved UV pump (4.77 eV) and VUV probe (7.94 eV) measurements of internal conversion of 1,3-cyclohexadiene (CHD). Our measurements reveal a substantial ionization of the "hot" ground state following internal conversion despite the fact that our probe photon energy is below the ionization potential (8.21 eV). With the aid of electronic structure calculations, we interpret our results in terms of vibrationally assisted below-threshold ionization, where vibrational energy is converted to electronic energy. The effect relies on both having vibrational modes which allow for this vibrational-electronic coupling and exciting these modes during the internal conversion. We contrast our measurements in CHD with another similar molecule, cis,cis-1,3-cyclooctadiene (cis,cis-COD), for which we do not see the effect.

  16. Theoretical IR spectra of ionized naphthalene

    NASA Technical Reports Server (NTRS)

    Pauzat, F.; Talbi, D.; Miller, M. D.; DeFrees, D. J.; Ellinger, Y.

    1992-01-01

    We report the results of a theoretical study of the effect of ionization on the IR spectrum of naphthalene, using ab initio molecular orbital theory. For that purpose we determined the structures, band frequencies, and intensities of neutral and positively ionized naphthalene. The calculated frequencies and intensities allowed an assignment of the most important bands appearing in the newly reported experimental spectrum of the positive ion. Agreement with the experimental spectrum is satisfactory enough to take into consideration the unexpected and important result that ionization significantly affects the intensities of most vibrations. A possible consequence on the interpretation of the IR interstellar emission, generally supposed to originate from polycyclic aromatic hydrocarbons (PAHs), is briefly presented.

  17. Streaking of shake-up ionization

    NASA Astrophysics Data System (ADS)

    Pazourek, Renate; Nagele, Stefan; Feist, Johannes; Kaltenbäck, Andreas; Persson, Emil; Schneider, Barry I.; Collins, Lee A.; Burgdörfer, Joachim

    2010-03-01

    We investigate whether an apparent ``time delay'' between electrons ionized by an attosecond XUV pulse with and without shake-up excitation of the remaining ion can be extracted using XUV-IR streaking setups. The classical interpretation of attosecond streaking states that the release time of an electron can be directly mapped to the momentum shift which the electron acquires from the IR pulse. However, detailed quantum mechanical investigations show that the ionization and shake-up process itself are modified by the IR field, leading to additional momentum shifts of the ionized electrons which are not related to a real ``time delay.'' We address this problem for the helium atom for which we solve the full time-dependent Schr"odinger equation including all correlation effects.

  18. Universal imaging: Dissociative ionization of polyatomic molecules, chemical dynamics beamline 9.0.2

    SciTech Connect

    Ahmed, M.; Chen, D.; Suits, A.G.

    1997-04-01

    A third endstation was recently added to the Chemical Dynamics beamline, designed to exploit the high flux broadband undulator light for a range of studies of reactive scattering, photochemistry and photoionization processes using time-of-flight mass spectroscopy coupled with position-sensitive detection. Two molecular beam sources are fixed at right angles, with the undulator light, or laser beams, intersecting the molecular beams at 45{degrees}. To date, beamline experiments have included a study of dissociative photoionization of a variety of molecules including N{sub 2}O and SF{sub 6}. In this mode, a single molecular beam source is used, with the tunable undulator light inducing, in SF{sub 6} for example, the process SF{sub 6} {r_arrow} SF{sub 6}{sup +} + e{sup {minus}} {r_arrow} SF{sub 5}{sup +} + F + e{sup {minus}}. The SF{sub 5}{sup +} ions are accelerated up the flight tube, mass selected and detected as a function of position on a phosphor screen viewed by a CCD camera. The position directly reveals the recoil speed (or translational energy release) and angular distribution for the dissociative ionization process. Furthermore, this measurement is obtained for all recoil speeds and angles simultaneously. Such detailed angular information has not previously been obtained for dissociative ionization processes; typically ion time-of-flight profiles are deconvoluted to yield rough insight into the angular distributions. The recorded image is actually a 2-dimensional projection of the nascent 3-dimensional velocity distribution, but established tomographic techniques enable the authors to reconstruct the 3-D distribution.

  19. Electrospray ionization of volatiles in breath

    NASA Astrophysics Data System (ADS)

    Martínez-Lozano, P.; de La Mora, J. Fernández

    2007-08-01

    Recent work by Zenobi and colleagues [H. Chen, A. Wortmann, W. Zhang, R. Zenobi, Angew. Chem. Int. Ed. 46 (2007) 580] reports that human breath charged by contact with an electrospray (ES) cloud yields many mass peaks of species such as urea, glucose, and other ions, some with molecular weights above 1000 Da. All these species are presumed to be involatile, and to originate from breath aerosols by so-called extractive electrospray ionization EESI [H. Chen, A. Venter, R.G. Cooks, Chem. Commun. (2006) 2042]. However, prior work by Fenn and colleagues [C.M. Whitehouse, F. Levin, C.K. Meng, J.B. Fenn, Proceedings of the 34th ASMS Conference on Mass Spectrometry and Allied Topics, Denver, 1986 p. 507; S. Fuerstenau, P. Kiselev, J.B. Fenn, Proceedings of the 47th ASMS Conference on Mass Spectrometry, 1999, Dallas, TX, 1999] and by Hill and colleagues [C. Wu, W.F. Siems, H.H. Hill Jr., Anal. Chem. 72 (2000) 396] have reported the ability of electrospray drops to ionize a variety of low vapor pressure substances directly from the gas phase, without an apparent need for the vapor to be brought into the charging ES in aerosol form. The Ph.D. Thesis of Martínez-Lozano [P. Martínez-Lozano Sinués, Ph.D. Thesis, Department of Thermal and Fluid Engineering, University Carlos III of Madrid; April 5, 2006 (in Spanish); http://hdl.handle.net/10016/655] had also previously argued that the numerous human breath species observed via a similar ES ionization approach were in fact ionized directly from the vapor. Here, we observe that passage of the breath stream through a submicron filter does not eliminate the majority of the breath vapors seen in the absence of the filter. We conclude that direct vapor charging is the leading mechanism in breath ionization by electrospray drops, though aerosol ionization may also play a role.

  20. Guided ionization waves: Theory and experiments

    NASA Astrophysics Data System (ADS)

    Lu, X.; Naidis, G. V.; Laroussi, M.; Ostrikov, K.

    2014-07-01

    This review focuses on one of the fundamental phenomena that occur upon application of sufficiently strong electric fields to gases, namely the formation and propagation of ionization waves-streamers. The dynamics of streamers is controlled by strongly nonlinear coupling, in localized streamer tip regions, between enhanced (due to charge separation) electric field and ionization and transport of charged species in the enhanced field. Streamers appear in nature (as initial stages of sparks and lightning, as huge structures-sprites above thunderclouds), and are also found in numerous technological applications of electrical discharges. Here we discuss the fundamental physics of the guided streamer-like structures-plasma bullets which are produced in cold atmospheric-pressure plasma jets. Plasma bullets are guided ionization waves moving in a thin column of a jet of plasma forming gases (e.g., He or Ar) expanding into ambient air. In contrast to streamers in a free (unbounded) space that propagate in a stochastic manner and often branch, guided ionization waves are repetitive and highly-reproducible and propagate along the same path-the jet axis. This property of guided streamers, in comparison with streamers in a free space, enables many advanced time-resolved experimental studies of ionization waves with nanosecond precision. In particular, experimental studies on manipulation of streamers by external electric fields and streamer interactions are critically examined. This review also introduces the basic theories and recent advances on the experimental and computational studies of guided streamers, in particular related to the propagation dynamics of ionization waves and the various parameters of relevance to plasma streamers. This knowledge is very useful to optimize the efficacy of applications of plasma streamer discharges in various fields ranging from health care and medicine to materials science and nanotechnology.

  1. New Results in Electron-Atom Ionization

    NASA Astrophysics Data System (ADS)

    Madison, Don

    1997-10-01

    A deeper insight into atomic ionization by electron impact is gained by studying electron-electron correlation in a model-independent approach for calculating (e,2e) triply-differential cross sections using correlated (three-body) wave functions of arbitrary complexity. Results will be presented from the continuum distorted wave (CDW) model, three Coulomb-wave (3C) model, three-body distorted-wave Born approximation (3DWBA), Alt and Mukhamedzhanov (AM) model, dynamic-screening three Coulomb-wave (DS3C) model, and the eikonal approximation (EA). The sucesses and failures of the above models can be used to gain a better understanding of ionization processes.

  2. Accreditation of ionizing radiation protection programs

    SciTech Connect

    McDonald, J.C.; Swinth, K.L.; Selby, J.M.

    1991-10-01

    There are over one million workers in the United States who have the potential to be exposed to ionizing radiation. Therefore, it is necessary to determine accurately the quantity of radiation to which they may have been exposed. This quantity if measured by personnel dosimeters that are carried by individuals requiring radiation monitoring. Accreditation of the organizations which evaluate this quantity provides official recognition of the competence of these organizations. Accreditation programs in the field of ionizing radiation protection have been in operation for a number of years, and their experience has demonstrated that such programs can help to improve performance.

  3. Effect of surface ionization on wetting layers

    NASA Technical Reports Server (NTRS)

    Kayser, R. F.

    1986-01-01

    A surface ionization model due to Langmuir is generalized to liquid mixtures of polar and nonpolar components in contact with ionizable substrates. When a predominantly nonpolar mixture is near a miscibility gap, thick wetting layers of the conjugate polar phase form on the substrate. Such charged layers can be much thicker than similar wetting layers stabilized by dispersion forces. This model may explain the 0.4- to 0.6-micron-thick wetting layers formed in stirred mixtures of nitromethane and carbon disulfide in contact with glass.

  4. Mechanism of branching in negative ionization fronts.

    PubMed

    Arrayás, Manuel; Fontelos, Marco A; Trueba, José L

    2005-10-14

    When a strong electric field is applied to nonconducting matter, narrow channels of plasma called streamers may form. Branchlike patterns of streamers have been observed in anode directed discharges. We explain a mechanism for branching as the result of a balance between the destabilizing effect of impact ionization and the stabilizing effect of electron diffusion on ionization fronts. The dispersion relation for transversal perturbation of a planar negative front is obtained analytically when the ratio D between the electron diffusion coefficient and the intensity of the externally imposed electric field is small. We estimate the spacing lambda between streamers and deduce a scaling law lambda approximately D(1/3).

  5. Electron-Impact Ionization Cross Section Database

    National Institute of Standards and Technology Data Gateway

    SRD 107 Electron-Impact Ionization Cross Section Database (Web, free access)   This is a database primarily of total ionization cross sections of molecules by electron impact. The database also includes cross sections for a small number of atoms and energy distributions of ejected electrons for H, He, and H2. The cross sections were calculated using the Binary-Encounter-Bethe (BEB) model, which combines the Mott cross section with the high-incident energy behavior of the Bethe cross section. Selected experimental data are included.

  6. Electron-impact ionization of ozone

    NASA Astrophysics Data System (ADS)

    Newson, Karl A.; Luc, Stephanie M.; Price, Stephen D.; Mason, Nigel J.

    1995-10-01

    Partial electron ionization cross-sections of ozone for incident electron energies from 40 to 500 eV have been determined using time-of-flight mass spectrometry. The cross-sections are derived by identifying the contribution of ozone to the ion signals recorded following ionization of a mixture of O2 and O3. Only one previous determination of these cross-sections, for energies up to 100 eV, is available in the literature. The cross-sections derived in the present study at these lower electron energies are in good agreement with the previous determination.

  7. Double ionization of helium by particle impact

    NASA Technical Reports Server (NTRS)

    Jacobsen, Finn M.

    1990-01-01

    Experimental results are reviewed of the ratio, R sq., of double to single ionization of He by proton, antiproton, electron and positron impact in the energy range from 0.15 to about 10 MeV/amu. At high velocities (greater than 1 to 2 MeV/amu) values of R sq. caused by electron impact merge with those for the proton with the antiproton, electron values being up to a factor of 2 greater than that for the p, positron. At these velocities the single ionization cross sections caused by impact of any of these four particles are indistinguishable.

  8. Femtosecond multiphoton ionization of ammonia clusters

    SciTech Connect

    Wei, S.; Purnell, J.; Buzza, S.A.; Stanley, R.J.; Castleman, A.W. Jr. )

    1992-12-15

    Herein, we report on femtosecond time-resolved experiments in ammonia clusters. The mechanisms of their ionization and the subsequent formation of the protonated ammonia cluster ions are studied using a femtosecond pump-probe technique at 620 nm. It is found that an intermediate corresponding to [ital C][prime] states of the monomer is responsible for the ionization of ammonia clusters. Femtosecond pump--probe studies show that the lifetime of the intermediate to the formation of the protonated cluster ions (NH[sub 3])[sub [ital n

  9. Dissociative Ionization of Pyridine by Electron Impact

    NASA Technical Reports Server (NTRS)

    Dateo, Christopher; Huo, Winifred; Kwak, Dochan (Technical Monitor)

    2002-01-01

    In order to understand the damage of biomolecules by electrons, a process important in radiation damage, we undertake a study of the dissociative ionization (DI) of pyridine (C5H5N) from the low-lying ionization channels. The methodology used is the same as in the benzene study. While no experimental DI data are available, we compare the dissociation products from our calculations with the dissociative photoionization measurements of Tixier et al. using dipole (e, e(+) ion) coincidence spectroscopy. Comparisons with the DI of benzene is also made so as to understand the difference in DI between a heterocyclic and an aromatic molecule.

  10. A prototype ionization profile monitor for RHIC

    SciTech Connect

    Connolly, R.; Cameron, P.; Ryan, W.

    1997-07-01

    Transverse beam profiles in the Relativistic Heavy-Ion Collider (RHIC) will be measured with ionization profile monitors (IPM`s). Each IPM collects and measures the distribution of electrons in the beamline resulting from residual gas ionization during bunch passage. The electrons are swept transversely from the beamline and collected on strip anodes oriented parallel to the beam axis. At each bunch passage the charge pulses are amplified, integrated, and digitized for display as a profile histogram. A prototype detector was tested in the injection line during the RHIC Sextant Test. This paper describes the detector and gives results from the beam tests.

  11. Electron Vortices in Femtosecond Multiphoton Ionization

    NASA Astrophysics Data System (ADS)

    Pengel, D.; Kerbstadt, S.; Johannmeyer, D.; Englert, L.; Bayer, T.; Wollenhaupt, M.

    2017-02-01

    Multiphoton ionization of potassium atoms with a sequence of two counter-rotating circularly polarized femtosecond laser pulses produces vortex-shaped photoelectron momentum distributions in the polarization plane describing Archimedean spirals. The pulse sequences are produced by polarization shaping and the three-dimensional photoelectron distributions are tomographically reconstructed from velocity map imaging measurements. We show that perturbative ionization leads to electron vortices with c6 rotational symmetry. A change from c6 to c4 rotational symmetry of the vortices is demonstrated for nonperturbative interaction.

  12. (Oncogenic action of ionizing radiation)

    SciTech Connect

    Not Available

    1990-01-01

    An extensive experiment involving approximately 400 rats exposed to the neon ion beam at the Bevalac in Berkeley, CA and to electrons is nearing completion. The carcinogenicity of energetic electrons was determined for comparison with the neon ion results. As in past reports we will describe progress in three areas corresponding to the specific aims of the proposal: (1) carcinogenesis and DNA strand breaks in rat skin following exposure by the neon ions or electrons; (2) DNA strand breaks in the epidermis as a function of radiation penetration; (3) oncogene activation in radiation-induced rat skin cancers. 72 refs., 6 tabs.

  13. Matrix assisted ionization in vacuum, a sensitive and widely applicable ionization method for mass spectrometry.

    PubMed

    Trimpin, Sarah; Inutan, Ellen D

    2013-05-01

    An astonishingly simple new method to produce gas-phase ions of small molecules as well as proteins from the solid state under cold vacuum conditions is described. This matrix assisted ionization vacuum (MAIV) mass spectrometry (MS) method produces multiply charged ions similar to those that typify electrospray ionization (ESI) and uses sample preparation methods that are nearly identical to matrix-assisted laser desorption/ionization (MALDI). Unlike these established methods, MAIV does not require a laser or voltage for ionization, and unlike the recently introduced matrix assisted ionization inlet method, does not require added heat. MAIV-MS requires only introduction of a crystalline mixture of the analyte incorporated with a suitable small molecule matrix compound such as 3-nitrobenzonitrile directly to the vacuum of the mass spectrometer. Vacuum intermediate pressure MALDI sources and modified ESI sources successfully produce ions for analysis by MS with this method. As in ESI-MS, ion formation is continuous and, without a laser, little chemical background is observed. MAIV, operating from a surface offers the possibility of significantly improved sensitivity relative to atmospheric pressure ionization because ions are produced in the vacuum region of the mass spectrometer eliminating losses associated with ion transfer from atmospheric pressure to vacuum. Mechanistic aspects and potential applications for this new ionization method are discussed.

  14. The Galactic Warm Ionized Medium: the First Direct Measures of its Ionization and Abundances

    NASA Astrophysics Data System (ADS)

    Howk, J.

    2002-07-01

    The warm ionized medium {WIM} is the dominant gaseous component of the Galactic halo and represents an important sink of the radiative and kinetic energy output of stars and supernovae, though the source of its ionization remains unknown. We will use stis spectroscopy of the post-AGB stars ROB 162 and ZNG 1 in the globular clusters NGC 6397 and Messier 5 to measure directly the abundances and ionization states of several key metals in the Galactic WIM. These sight lines are unique: because the two clusters also contain pulsars with published radio dispersion measurements, these are the only sight lines for which we can derive the column densities of both HI, em and ionH2, as well as the columns of multiple ionization stages of the important metals S, P, and Fe. We will use the proposed stis observations with existing Ause data to derive the total gas-phase abundances of S, P, and Fe for the material along these sight lines with no ionization uncertainties. We will directly measure the ionization fractions of S and P in the WIM. We will also infer the dust content of the WIM. Our study of the ionization state and dust content of the WIM will provide the best yet constraints for models of this gas. Our work will also provide the best constraint for the fundamental ``cosmic'' reference abundance {averaged over these sight lines} of the undepleted elements S and P.

  15. Electron capture by U(91+) and U(92+) and ionization of U(90+) and U(91+)

    NASA Technical Reports Server (NTRS)

    Gould, H.; Greiner, D.; Lindstrom, P.; Symons, T. J. M.; Crawford, H.

    1984-01-01

    U(92+)/U(91+) and U(91+)/U(90+) electron-capture and ionization cross sections and equilibrium charge-state distributions are measured experimentally in mylar, Cu and Ta of varying thickness. Relativistic U(68+) ions at 437 or 962 MeV/nucleon are produced by a heavy-ion linear accelerator and synchrotron in tandem and passed through the target material into a magnetic specrometer and position-sensitive proportional counter for evaluation of charge states. The results are presented graphically and discussed. At 962 MeV/nucleon, beams containing 85 percent bare U(92+) nuclei are obtained using 150-mg/sq cm Cu or 85-mg/sq cm Ta; at 437 MeV/nucleon, 50 percent bare U(92+) nuclei are obtained with 90-mg/sq cm Cu. The techniques decribed can be applied to produce beams of bare U nuclei for acceleration to ultrarelativistic speeds or beams of few-electron U for atomic-physics experiments on quantum electrodynamics.

  16. Electron capture by U(91+) and U(92+) and ionization of U(90+) and U(91+)

    NASA Technical Reports Server (NTRS)

    Gould, H.; Greiner, D.; Lindstrom, P.; Symons, T. J. M.; Crawford, H.

    1984-01-01

    U(92+)/U(91+) and U(91+)/U(90+) electron-capture and ionization cross sections and equilibrium charge-state distributions are measured experimentally in mylar, Cu and Ta of varying thickness. Relativistic U(68+) ions at 437 or 962 MeV/nucleon are produced by a heavy-ion linear accelerator and synchrotron in tandem and passed through the target material into a magnetic specrometer and position-sensitive proportional counter for evaluation of charge states. The results are presented graphically and discussed. At 962 MeV/nucleon, beams containing 85 percent bare U(92+) nuclei are obtained using 150-mg/sq cm Cu or 85-mg/sq cm Ta; at 437 MeV/nucleon, 50 percent bare U(92+) nuclei are obtained with 90-mg/sq cm Cu. The techniques decribed can be applied to produce beams of bare U nuclei for acceleration to ultrarelativistic speeds or beams of few-electron U for atomic-physics experiments on quantum electrodynamics.

  17. Liquid Heparin Anticoagulant Produces More Negative Bias in the Determination of Ionized Magnesium than Ionized Calcium

    PubMed Central

    Shin, Cheung Soo; Chang, Chul Ho

    2006-01-01

    The ionized calcium level in blood is known to be falsely decreased when self-prepared liquid heparin anticoagulant is used, due to dilution and binding effects. The effect of liquid heparin on the determination of ionized magnesium is not as well understood. We compared the effect of liquid sodium heparin on the determination of ionized calcium and magnesium in 44 clinical samples using two types of user-prepared heparin syringes which differed in the amount of residual heparin from the BD Preset™ reference syringe. With the type 1 syringe, the liquid heparin was expelled once or twice such that some heparin could be left in the dead space at the syringe hub, while the liquid sodium heparin was thoroughly expelled from the type 2 syringe. The ionized magnesium levels obtained with the type 1 syringe were significantly lower than the reference value (by 0.068 mmol/L) (p < 0.0001), while the value obtained with the type 2 syringe differed less from the reference, by only 0.014 mmol/L (p < 0.0001). The heparin binding effect resulted in more negative bias in ionized magnesium (- 0.026 ± 0.032 mmol/L) than in ionized calcium (- 0.009 ± 0.042 mmol/L, p < 0.0001). In conclusion, we recommend using lyophilized, calcium-balanced, heparinized syringes for the determination of ionized magnesium and ionized calcium due to the increased negative bias in ionized magnesium determinations. When user-prepared syringes are used, the thorough evacuation of heparin solution should be strictly prescribed. PMID:16642547

  18. Ionization states in the microenvironment of solid dosage forms: effect of formulation variables and processing.

    PubMed

    Govindarajan, Ramprakash; Zinchuk, Andrey; Hancock, Bruno; Shalaev, Evgenyi; Suryanarayanan, Raj

    2006-10-01

    Evaluation of the effect of formulation composition and processing variables on the microenvironment in solid dosage forms, based on ionization of indicator probes. Sulfonephthalein indicators were intimately mixed with individual excipients, binary excipient mixtures or multi-component blends by the solvent deposition method. Diffuse reflectance visible spectroscopy of these solids provided a measure of indicator ionization extent. Indicator solution studies yielded equations relating solution pH to the ratio of the absorbance signals of the ionized to that of the unionized form, for each indicator. These equations and the spectral data of the indicator-treated solids were used to calculate an acidity function, 'pH(eq)' for the solids. The ionization of incorporated probes was also monitored during various stages of simulated pharmaceutical processing viz. wet and dry mixing. The pH(eq) provided a measure of the physicochemical environment experienced by the probe in the solid. The surface nature of formulation components and their surface area available for interaction influenced the overall properties of the final blend. The extent of probe ionization varied at different stages of a simulated wet mixing-drying process. The pH of the excipient suspension was not a good predictor of the probe ionization in the final dried solid. Indicator ionization is expected to be influenced by the microenvironmental acidity, polarity and ionic strength. Individual excipient properties contributed to the overall microenvironment in powder mixtures even when dry mixed at low water contents. The environment experienced by a drug in the final solid dosage form will be influenced by the nature of the excipients, the extent of their surfaces available for interaction, surface modification during processing and the amount and nature of solvent used.

  19. Ejection-ionization of molecules from free standing graphene

    NASA Astrophysics Data System (ADS)

    Verkhoturov, Stanislav V.; Czerwinski, Bartlomiej; Verkhoturov, Dmitriy S.; Geng, Sheng; Delcorte, Arnaud; Schweikert, Emile A.

    2017-02-01

    We present the first data on emission of -C60 stimulated by single impacts of 50 keV C60+2 on the self-assembled molecular layer of C60 deposited on free standing 2 layer graphene. The yield, Y, of -C60 emitted in the transmission direction is 1.7%. To characterize the ejection and ionization of molecules, we have measured the emission of -C60 from the surface of bulk C60 (Y = 3.7%) and from a single layer of C60 deposited on bulk pyrolytic graphite (Y = 3.3%). To gain insight into the mechanism(s) of ejection, molecular dynamic simulations were performed. The scenario of the energy deposition and ejection of molecules is different for the case of graphene due to the confined volume of projectile-analyte interaction. In the case of 50 keV C60+2 impacts on graphene plus C60, the C atoms of the projectile collide with those of the target. The knocked-on atoms take on a part of the kinetic energy of the projectile atoms. Another part of the kinetic energy is deposited into the rim around the impact site. The ejection of molecules from the rim is a result of collective movement of the molecules and graphene membrane, where the membrane movement provides the impulse for ejection. The efficient emission of the intact molecular ions implies an effective ionization probability of intact C60. The proposed mechanism of ionization involves the tunneling of electrons from the vibrationally exited area around the hole to the ejecta.

  20. Composite scintillators for detection of ionizing radiation

    DOEpatents

    Dai, Sheng [Knoxville, TN; Stephan, Andrew Curtis [Knoxville, TN; Brown, Suree S [Knoxville, TN; Wallace, Steven A [Knoxville, TN; Rondinone, Adam J [Knoxville, TN

    2010-12-28

    Applicant's present invention is a composite scintillator having enhanced transparency for detecting ionizing radiation comprising a material having optical transparency wherein said material comprises nano-sized objects having a size in at least one dimension that is less than the wavelength of light emitted by the composite scintillator wherein the composite scintillator is designed to have selected properties suitable for a particular application.

  1. Dissociative Ionization of Benzene by Electron Impact

    NASA Technical Reports Server (NTRS)

    Huo, Winifred; Dateo, Christopher; Kwak, Dochan (Technical Monitor)

    2002-01-01

    We report a theoretical study of the dissociative ionization (DI) of benzene from the low-lying ionization channels. Our approach makes use of the fact that electron motion is much faster than nuclear motion and DI is treated as a two-step process. The first step is electron-impact ionization resulting in an ion with the same nuclear geometry as the neutral molecule. In the second step the nuclei relax from the initial geometry and undergo unimolecular dissociation. For the ionization process we use the improved binary-encounter dipole (iBED) model. For the unimolecular dissociation step, we study the steepest descent reaction path to the minimum of the ion potential energy surface. The path is used to analyze the probability of unimolecular dissociation and to determine the product distributions. Our analysis of the dissociation products and the thresholds of the productions are compared with the result dissociative photoionization measurements of Feng et al. The partial oscillator strengths from Feng et al. are then used in the iBED cross section calculations.

  2. Liquid-filled ionization chamber temperature dependence

    NASA Astrophysics Data System (ADS)

    Franco, L.; Gómez, F.; Iglesias, A.; Pardo, J.; Pazos, A.; Pena, J.; Zapata, M.

    2006-05-01

    Temperature and pressure corrections of the read-out signal of ionization chambers have a crucial importance in order to perform high-precision absolute dose measurements. In the present work the temperature and pressure dependences of a sealed liquid isooctane filled ionization chamber (previously developed by the authors) for radiotherapy applications have been studied. We have analyzed the thermal response of the liquid ionization chamber in a ˜20C interval around room temperature. The temperature dependence of the signal can be considered linear, with a slope that depends on the chamber collection electric field. For example, a relative signal slope of 0.27×10-2 K-1 for an operation electric field of 1.67×106 V m-1 has been measured in our detector. On the other hand, ambient pressure dependence has been found negligible, as expected for liquid-filled chambers. The thermal dependence of the liquid ionization chamber signal can be parametrized within the Onsager theory on initial recombination. Considering that changes with temperature of the detector response are due to variations in the free ion yield, a parametrization of this dependence has been obtained. There is a good agreement between the experimental data and the theoretical model from the Onsager framework.

  3. Applying the helium ionization detector in chromatography

    NASA Technical Reports Server (NTRS)

    Gibson, E. K.; Andrawes, F. F.; Brazell, R. S.

    1981-01-01

    High noise levels and oversensitivity of helium detector make flame-ionization and thermal-conductivity detectors more suitable for chromotography. Deficiencies are eliminated by modifying helium device to operate in saturation rather than multiplication mode. Result is low background current, low noise, high stability, and high sensitivity. Detector analyzes halocarbons, hydrocarbons, hydrogen cyanide, ammonia, and inorganics without requiring expensive research-grade helium.

  4. Relativistic soliton-like collisionless ionization wave

    NASA Astrophysics Data System (ADS)

    Arefiev, Alexey; McCormick, Matthew; Quevedo, Hernan; Bengtson, Roger; Ditmire, Todd

    2014-10-01

    It has been observed in recent experiments with laser-irradiated gas jets that a plasma filament produced by the laser and containing energetic electrons can launch a relativistic ionization wave into ambient gas. Here we present a self-consistent theory that explains how a collisionless ionization wave can propagate in a self-sustaining regime. A population of hot electrons necessarily generates a sheath electric field at the plasma boundary. This field penetrates the ambient gas, ionizing the gas atoms and thus causing the plasma boundary to expand. We show that the motion of the newly generated electrons can form a potential well adjacent to the plasma boundary. The outwards motion of the well causes a bunch of energetic electrons to become trapped, while allowing the newly generated electrons to escape into the plasma without retaining much energy. The resulting soliton-like ionizing field structure propagates outwards with a bunch of hot electrons that maintain a strong sheath field despite significant plasma expansion. We also present 1D and 2D particle-in-cell simulations that illustrate the described mechanism. The simulations were performed using HPC resources provided by the Texas Advanced Computing Center. This work was supported by NNSA Contract No. DE-FC52-08NA28512 and U.S. DOE Contract No. DE-FG02-04ER54742.

  5. Ionization Energy: Implications of Preservice Teachers' Conceptions

    ERIC Educational Resources Information Center

    Tan, Kim Chwee Daniel; Taber, Keith S.

    2009-01-01

    The results from a study to explore pre-service teachers' understanding of ionization energy, a topic that features in A-level (grade 11 and 12) chemistry courses. in Singapore , is described. A previous study using a two-tier multiple choice diagnostic test has shown that Singapore A-level students have considerable difficulty understanding the…

  6. The MICE Demonstration of Muon Ionization Cooling

    SciTech Connect

    Lagrange, Jean-Baptiste; Hunt, Christopher; Palladino, Vittorio; Pasternak, Jaroslaw

    2016-06-01

    Muon beams of low emittance provide the basis for the intense, well-characterised neutrino beams necessary to elucidate the physics of flavour at the Neutrino Factory and to provide lepton-antilepton collisions up to several TeV at the Muon Collider. The international Muon Ionization Cooling Experiment (MICE) will demonstrate muon ionization cooling, the technique proposed to reduce the phase-space volume occupied by the muon beam at such facilities. In an ionization-cooling channel, the muon beam traverses a material (the absorber) loosing energy, which is replaced using RF cavities. The combined effect is to reduce the transverse emittance of the beam (transverse cooling). The configuration of MICE required to deliver the demonstration of ionization cooling is being prepared in parallel to the execution of a programme designed to measure the cooling properties of liquid-hydrogen and lithium hydride. The design of the cooling-demonstration experiment will be presented together with a summary of the performance of each of its components and the cooling performance of the experiment.

  7. Ionizing Radiation and Chronic Lymphocytic Leukemia

    PubMed Central

    Richardson, David B.; Wing, Steve; Schroeder, Jane; Schmitz-Feuerhake, Inge; Hoffmann, Wolfgang

    2005-01-01

    The U.S. government recently implemented rules for awarding compensation to individuals with cancer who were exposed to ionizing radiation while working in the nuclear weapons complex. Under these rules, chronic lymphocytic leukemia (CLL) is considered to be a nonradiogenic form of cancer. In other words, workers who develop CLL automatically have their compensation claim rejected because the compensation rules hold that the risk of radiation-induced CLL is zero. In this article we review molecular, clinical, and epidemiologic evidence regarding the radiogenicity of CLL. We note that current understanding of radiation-induced tumorigenesis and the etiology of lymphatic neoplasia provides a strong mechanistic basis for expecting that ionizing radiation exposure increases CLL risk. The clinical characteristics of CLL, including prolonged latency and morbidity periods and a low case fatality rate, make it relatively difficult to evaluate associations between ionizing radiation and CLL risk via epidemiologic methods. The epidemiologic evidence of association between external exposure to ionizing radiation and CLL is weak. However, epidemiologic findings are consistent with a hypothesis of elevated CLL mortality risk after a latency and morbidity period that spans several decades. Our findings in this review suggest that there is not a persuasive basis for the conclusion that CLL is a nonradiogenic form of cancer. PMID:15626639

  8. WARPED IONIZED HYDROGEN IN THE GALAXY

    SciTech Connect

    Cersosimo, J. C.; Figueroa, N. Santiago; Velez, S. Figueroa; Soto, C. Lozada; Mader, S.; Azcarate, D.

    2009-07-01

    We report observations of the H166{alpha} ({nu} = 1424.734 MHz) radio recombination line (RRL) emission from the Galactic plane in the longitude range l = 267 deg. - 302 deg. and latitude range b = -3.{sup 0}0 to +1.{sup 0}5. The line emission observed describes the Carina arm in the Galactic azimuth range from {theta} = 260 deg. to 190 deg. The structure is located at negative latitudes with respect to the formal Galactic plane. The observations are combined with RRL data from the first Galactic quadrant. Both quadrants show the signature of the warp for the ionized gas, but an asymmetry of the distribution is noted. In the fourth quadrant, the gas is located between Galactic radii R {approx} 7 and 10 kpc, and the amplitude of the warp is seen from the midplane to z {approx} -150 pc. In the first quadrant, the gas is found between R {approx} 8 and 13-16 kpc, and flares to z {approx} +350 pc. We confirm the warp of the ionized gas near the solar circle. The distribution of the ionized gas is compared with the maximum intensity H I emission (0.30 < n{sub HI} < 0.45 cm{sup -3}) at intervals of the Galactic ring. The ionized material is correlated with the H I maximum intensity in both quadrants, and both components show the same tilted behavior with respect to the mid-Galactic plane.

  9. Electron-impact ionization of W25+

    NASA Astrophysics Data System (ADS)

    Kynienė, A.; Pakalka, S.; Masys, Š.; Jonauskas, V.

    2016-09-01

    Electron-impact ionization cross sections for the ground level of the W25+ ion have been investigated by performing level-to-level calculations and using the Dirac-Fock-Slater method in the single-configuration approach. The main attention has been focused on the influence of the increasing principal and orbital quantum numbers on the excitation-autoionization (EA) process and its contribution to the total ionization cross sections. The obtained results demonstrate that excitations to the high-nl shells (n≥slant 9) increase cross sections of the indirect ionization process by about 60% compared to the excitations to the lower shells (n≤slant 8). It was established that excitations to the shells with the orbital quantum number l = 4 give the greatest contribution to EA. Maxwellian rate coefficients derived from the cross sections for the ground state are compared with the previously obtained values from the configuration-average distorted-wave (CADW) approximation. The rate coefficients for direct ionization (DI) are smaller than the corresponding CADW values, while the EA rate coefficients are larger than the ones from the CADW calculations. The total DI+EA rate coefficients are about 20% larger than the CADW rate coefficients.

  10. Limits to Sensitivity in Laser Enhanced Ionization.

    ERIC Educational Resources Information Center

    Travis, J. C.

    1982-01-01

    Laser enhanced ionization (LEI) occurs when a tunable dye laser is used to excite a specific atomic population in a flame. Explores the origin of LEI's high sensitivity and identifies possible avenues to higher sensitivity by describing instrument used and experimental procedures and discussing ion formation/detection. (Author/JN)

  11. Historical survey of resonance ionization spectroscopy

    SciTech Connect

    Hurst, G.S.

    1984-04-01

    We have recently celebrated the 10th birthday of Resonance Ionization Spectroscopy (RIS), and this seems an appropriate time to review the history of its development. Basically, RIS is a photophysics process in which tunable light sources are used to remove a valence electron from an atom of selected atomic number, Z. If appropriate lasers are used as the light source, one electron can be removed from each atom of the selected Z in the laser pulse. This implies that RIS can be a very efficient, as well as selective, ionization process. In what we normally call RIS, laser schemes are employed which preserve both of these features. In contrast, multiphoton ionization (MPI) is more general, although not necessarily Z selective or very efficient because resonances are often not used. Early research completed in the USSR and described as selective two-step photoionization, employed resonances to ionize the rubidium atom and served to guide work on laser isotope separation. 29 references, 8 figures.

  12. Salt Tolerance of Desorption Electrospray Ionization (DESI)

    SciTech Connect

    Jackson, Ayanna U.; Talaty, Nari; Cooks, R G; Van Berkel, Gary J

    2007-01-01

    Suppression of ion intensity in the presence of high salt matrices is common in most mass spectrometry ionization techniques. Desorption electrospray ionization (DESI) is an ionization method that exhibits salt tolerance, and this is investigated. DESI analysis was performed on three different drug mixtures in the presence of 0, 0.2, 2, 5, 10, and 20% NaCl:KCl weight by volume from seven different surfaces. At physiological concentrations individual drugs in each mixture were observed with each surface. Collision-induced dissociation (CID) was used to provide additional confirmation for select compounds. Multiple stage experiments, to MS5, were performed for select compounds. Even in the absence of added salt, the benzodiazepine containing mixture yielded sodium and potassium adducts of carbamazepine which masked the ions of interest. These adducts were eliminated by adding 0.1% 7M ammonium acetate to the standard methanol:water (1:1) spray solvent. Comparison of the salt tolerance of DESI with that of electrospray ionization (ESI) demonstrated much better signal/noise characteristics for DESI in this study. The salt tolerance of DESI was also studied by performing limit of detection and dynamic range experiments. Even at a salt concentration significantly above physiological concentrations, select surfaces were effective in providing spectra that allowed the ready identification of the compounds of interest. The already high salt tolerance of DESI can be optimized further by appropriate choices of surface and spray solution.

  13. Ionization Energy: Implications of Preservice Teachers' Conceptions

    ERIC Educational Resources Information Center

    Tan, Kim Chwee Daniel; Taber, Keith S.

    2009-01-01

    The results from a study to explore pre-service teachers' understanding of ionization energy, a topic that features in A-level (grade 11 and 12) chemistry courses. in Singapore , is described. A previous study using a two-tier multiple choice diagnostic test has shown that Singapore A-level students have considerable difficulty understanding the…

  14. Roles of ionizing radiation in cell transformation

    SciTech Connect

    Tobias, C.A.; Albright, N.W.; Yang, T.C.

    1983-07-01

    Earlier the authors described a repair misrepair model (RMR-I) which is applicable for radiations of low LET, e.g., x rays and gamma rays. RMR-II was described later. Here is introduced a mathematical modification of the RMR model, RMR-III, which is intended to describe lethal effects caused by heavily ionizing tracks. 31 references, 4 figures.

  15. Conduction in fully ionized liquid metals

    NASA Technical Reports Server (NTRS)

    Stevenson, D. J.; Ashcroft, N. W.

    1973-01-01

    Electron transport is considered in high density fully ionized liquid metals. Ionic structure is described in terms of hard-sphere correlation functions and the scattering is determined from self-consistently screened point ions. Applications to the physical properties of the deep interior of Jupiter are briefly considered.

  16. Conduction in fully ionized liquid metals

    NASA Technical Reports Server (NTRS)

    Stevenson, D. J.; Ashcroft, N. W.

    1974-01-01

    Electron transport is considered in high-density fully ionized liquid metals. Ionic structure is described in terms of hard-sphere-correlation functions and the scattering is determined from self-consistently screened point ions. Applications to the physical properties of the deep interior of Jupiter are briefly considered.

  17. Collisional Ionization Equilibrium for Optically Thin Plasmas

    NASA Technical Reports Server (NTRS)

    Bryans, P.; Mitthumsiri, W.; Savin, D. W.; Badnell, N. R.; Gorczyca, T. W.; Laming, J. M.

    2006-01-01

    Reliably interpreting spectra from electron-ionized cosmic plasmas requires accurate ionization balance calculations for the plasma in question. However, much of the atomic data needed for these calculations have not been generated using modern theoretical methods and their reliability are often highly suspect. We have utilized state-of-the-art calculations of dielectronic recombination (DR) rate coefficients for the hydrogenic through Na-like ions of all elements from He to Zn. We have also utilized state-of-the-art radiative recombination (RR) rate coefficient calculations for the bare through Na-like ions of all elements from H to Zn. Using our data and the recommended electron impact ionization data of Mazzotta et al. (1998), we have calculated improved collisional ionization equilibrium calculations. We compare our calculated fractional ionic abundances using these data with those presented by Mazzotta et al. (1998) for all elements from H to Ni, and with the fractional abundances derived from the modern DR and RR calculations of Gu (2003a,b, 2004) for Mg, Si, S, Ar, Ca, Fe, and Ni.

  18. Atmospheric Pressure Chemical Ionization Sources Used in The Detection of Explosives by Ion Mobility Spectrometry

    SciTech Connect

    Waltman, Melanie J.

    2010-05-01

    Explosives detection is a necessary and wide spread field of research. From large shipping containers to airline luggage, numerous items are tested for explosives every day. In the area of trace explosives detection, ion mobility spectrometry (IMS) is the technique employed most often because it is a quick, simple, and accurate way to test many items in a short amount of time. Detection by IMS is based on the difference in drift times of product ions through the drift region of an IMS instrument. The product ions are created when the explosive compounds, introduced to the instrument, are chemically ionized through interactions with the reactant ions. The identity of the reactant ions determines the outcomes of the ionization process. This research investigated the reactant ions created by various ionization sources and looked into ways to manipulate the chemistry occurring in the sources.

  19. Effect of sample compositions on chemical analysis using matrix-assisted laser desorption ionization mass spectrometry

    NASA Astrophysics Data System (ADS)

    Schriemer, David; Dai, Yuqin; Li, Liang

    1996-11-01

    Matrix-assisted laser desorption ionization (MALDI) is an effective ionization technique for mass spectrometry. It take advantages of some unique properties of certain organic chemicals to provide entrapment, isolation, vaporization, and ionization of the analyte of interest. While the main application of the MALDI technique is currently in the area of biological molecule analysis, it is possible to use this technique for monitoring polymer chemistry such as degradation processes. This is potentially important for studying and developing environmentally degradable polymers. Direct analysis of the analyte in real-world samples is possible with MALDI. However, there is a significant effect of the overall composition of a sample on the detectability and performance of MALDI. Two examples are given to illustrate the positive and negative effects of buffers, salts, and additives on the MALDI sample preparation.

  20. Design of a secondary ionization target for direct production of a C(-) beam from CO2 pulses for online AMS.

    PubMed

    Salazar, Gary; Ognibene, Ted

    2013-01-01

    We designed and optimized a novel device "target" that directs a CO2 gas pulse onto a Ti surface where a Cs(+) beam generates C(-) from the CO2. This secondary ionization target enables an accelerator mass spectrometer to ionize pulses of CO2 in the negative mode to measure (14)C/(12)C isotopic ratios in real time. The design of the targets were based on computational flow dynamics, ionization mechanism and empirical optimization. As part of the ionization mechanism, the adsorption of CO2 on the Ti surface was fitted with the Jovanovic-Freundlich isotherm model using empirical and simulation data. The inferred adsorption constants were in good agreement with other works. The empirical optimization showed that amount of injected carbon and the flow speed of the helium carrier gas improve the ionization efficiency and the amount of (12)C(-) produced until reaching a saturation point. Linear dynamic range between 150 and 1000 ng of C and optimum carrier gas flow speed of around 0.1 mL/min were shown. It was also shown that the ionization depends on the area of the Ti surface and Cs(+) beam cross-section. A range of ionization efficiency of 1-2.5% was obtained by optimizing the described parameters.

  1. Nucleation in an Ultra Low Ionization Environment

    NASA Astrophysics Data System (ADS)

    Pedersen, J. O.; Enghoff, M. B.; Paling, S.; Svensmark, H.

    2010-12-01

    Atmospheric ions can enhance the nucleation of aerosols, as has been established by experiments, observation, and theory. In the clean marine atmosphere ionization is mainly caused by cosmic rays which in turn are controlled by the activity of the Sun, thus providing a potential link between solar activity and climate. In order to understand the effect ions may have on the production of cloud condensation nuclei the overall contribution of ion induced nucleation to the global production of secondary aerosols must be determined. One issue with determining this contribution is that several mechanisms for nucleation exist and it can be difficult to determine the relative importance of the various mechanisms in a given nucleation event when both ion induced and electrically neutral nucleation mechanisms are at work at the same time. We have carried out nucleation experiments in the Boulby Underground Laboratory, located 1100 meters below ground, thus reducing the flux of ionizing cosmic radiation by six orders of magnitude. Similarly we have reduced the gamma background by shielding the experiment in lead and copper. Finally we have used air stored for several weeks and passed through an active charcoal filter in order to reduce the Radon concentration. In this way we have been able to make nucleation experiments with very low ionizing background, meaning that we can rule out ion induced nucleation as a contributing mechanism. Our experimental setup is a 50 L electropolished stainless steel reactor at near atmospheric conditions. The chamber contains clean air with the addition of water vapor, ozone, and SO2. Using UV lights at 254 nm ozone is photolyzed, leading to the production of sulfuric acid and thus aerosols. An 18 MBq Caesium-137 gamma ray source with various amounts of lead in front allows us to alter the ionization in our chamber. By making series of nucleation bursts with varying amounts of ionizing radiation we then gauge the relative importance of ion

  2. Venturi easy ambient sonic-spray ionization.

    PubMed

    Santos, Vanessa G; Regiani, Thaís; Dias, Fernanda F G; Romão, Wanderson; Jara, Jose Luis Paz; Klitzke, Clécio F; Coelho, Fernando; Eberlin, Marcos N

    2011-02-15

    The development and illustrative applications of an ambient ionization technique termed Venturi easy ambient sonic-spray ionization (V-EASI) is described. Its dual mode of operation with Venturi self-pumping makes V-EASI applicable to the direct mass spectrometric analysis of both liquid (V(L)-EASI) and solid (V(S)-EASI) samples. V-EASI is simple and easy to assemble, operating solely via the assistance of a sonic stream of nitrogen or air. The sonic gas stream causes two beneficial and integrated effects: (a) the self-pumping of solutions via the Venturi effect and (b) sonic-spray ionization (SSI) of analytes either in solution or resting on solid surfaces. In its liquid mode, V(L)-EASI is applicable to analytes in solution, forming negatively and/or positively charged intact molecular species in a soft fashion with little or no fragmentation. In its solid mode, V(S)-EASI relies on Venturi self-pumping of a proper SSI solvent solution in combination with SSI to form a stream of bipolar charged droplets that bombard the sample surface, causing desorption and ionization of the analyte molecules. As for its precursor technique (EASI), V-EASI generates bipolar droplets with considerably lower average charging, which increases selectivity for ionization with high signal-to-noise ratios and clean spectra dominated by single molecular species with minimal solvent ions. V-EASI also operates in a voltage-, heat-, and radiation-free fashion and is therefore free of thermal, electrical, or discharge interferences.

  3. Ionization of amphiphilic acidic block copolymers.

    PubMed

    Colombani, Olivier; Lejeune, Elise; Charbonneau, Céline; Chassenieux, Christophe; Nicolai, Taco

    2012-06-28

    The ionization behavior of an amphiphilic diblock copolymer poly(n-butyl acrylate(50%)-stat-acrylic acid(50%))(100)-block-poly(acrylic acid)(100) (P(nBA(50%)-stat-AA(50%))(100)-b-PAA(100), DH50) and of its equivalent triblock copolymer P(nBA(50%)-stat-AA(50%))(100)-b-PAA(200)-b-P(nBA(50%)-stat-AA(50%))(100) (TH50) were studied by potentiometric titration either in pure water or in 0.5 M NaCl. These polymers consist of a hydrophilic acidic block (PAA) connected to a hydrophobic block, P(nBA(50%)-stat-AA(50%))(100), whose hydrophobic character has been mitigated by copolymerization with hydrophilic units. We show that all AA units, even those in the hydrophobic block could be ionized. However, the AA units within the hydrophobic block were less acidic than those in the hydrophilic block, resulting in the preferential ionization of the latter block. The preferential ionization of PAA over that of P(nBA(50%)-stat-AA(50%))(100) was stronger at higher ionic strength. Remarkably, the covalent bonds between the PAA and P(nBA(50%)-stat-AA(50%))(100) blocks in the diblock or the triblock did not affect the ionization of each block, although the self-association of the block copolymers into spherical aggregates modified the environment of the PAA blocks compared to when PAA was molecularly dispersed.

  4. Resonance-mediated atomic ionization dynamics induced by ultraintense x-ray pulses

    SciTech Connect

    Ho, Phay J.; Kanter, E. P.; Young, L.

    2015-12-31

    We describe the methodology of our recently developed Monte Carlo rate equation (MCRE) approach, which systematically incorporates bound-bound resonances to model multiphoton ionization dynamics induced by high-fluence, high-intensity x-ray free-electron laser (XFEL) pulses. These resonances are responsible for ionization far beyond that predicted by the sequential single photon absorption model and are central to a quantitative understanding of atomic ionization dynamics in XFEL pulses. We also present calculated multiphoton ionization dynamics for Kr and Xe atoms in XFEL pulses for a variety of conditions, to compare the effects of bandwidth, pulse duration, pulse fluence, and photon energy. This comprehensive computational investigation reveals areas in the photon energy–pulse fluence landscape where resonances are critically important. We also uncover a mechanism, preservation of inner-shell vacancies (PIVS), whereby radiation damage is enhanced at higher XFEL intensities and identify the sequence of core-outer–Rydberg, core-valence, and core-core resonances encountered during multiphoton x-ray ionization.

  5. Analytical procedures to identify foods that have been treated with ionizing radiation

    SciTech Connect

    Morehouse, K.M.

    1994-12-31

    Foods can be treated with ionizing radiation to reduce microbial infection and insect infestations, inhibit sprouting, and delay maturation, thereby extending the shelf life of foods. The treatment of different types of foods with ionizing radiation for specific purposes is accepted in several countries, although it is prohibited in others. The U.S. Food and Drug Administration (FDA) has established regulations to allow the treatment of several different foods with ionizing radiation and has received petitions for the approval of radiation treatment of additional foods. When carried out according to established good manufacturing practices, food irradiation yields safe, wholesome foods. Often, the irradiated product may be chemically and/or microbiologically {open_quotes}safer{close_quotes} than the nonirradiated product. An area of great interest in the last several years has been the development of analytical techniques to monitor foods that have been treated with ionizing radiation. A method for the identification of irradiated foods will help to foster compliance with labeling regulations, strengthen national and international regulations for the irradiation of specific foods, and enhance consumer confidence in the safety of food commodities that have been treated with ionizing radiation.

  6. Whether ionizing radiation is a risk factor for schizophrenia spectrum disorders?

    PubMed

    Loganovsky, Konstantin N; Volovik, Sergij V; Manton, Kenneth G; Bazyka, Dimitry A; Flor-Henry, Pierre

    2005-01-01

    The neural diathesis-stressor hypothesis of schizophrenia, where neurobiological genetic predisposition to schizophrenia can be provoked by environmental stressors is considered as a model of the effects of exposure to ionizing radiation. Analysis of information from electronic databases (MEDLINE, PsycINFO, EMBASE, Current Contents, Elsevier BIOBASE) and hand-made search was carried out. There are comparable reports on increases in schizophrenia spectrum disorders following exposure to ionizing radiation as a result of atomic bombing, nuclear weapons testing, the Chernobyl accident, environmental contamination by radioactive waste, radiotherapy, and also in areas with high natural radioactive background. The results of experimental radioneurobiological studies support the hypothesis of schizophrenia as a neurodegenerative disease. Exposure to ionizing radiation causes brain damage with limbic (cortical-limbic) system dysfunction and impairment of informative processes at the molecular level that can trigger schizophrenia in predisposed individuals or cause schizophrenia-like disorders. It is supposed that ionizing radiation can be proposed as a risk factor for schizophrenia spectrum disorders. The hypothesis that ionizing radiation is a risk factor for schizophrenia spectrum disorders can be tested using data from the Chernobyl accident aftermath. Implementation of a study on schizophrenia spectrum disorders in Chernobyl accident victims is of significance for both clinical medicine and neuroscience.

  7. Optimization of the ionization time of an atom with tailored laser pulses: a theoretical study

    NASA Astrophysics Data System (ADS)

    Kammerlander, David; Castro, Alberto; Marques, Miguel A. L.

    2017-05-01

    How fast can a laser pulse ionize an atom? We address this question by considering pulses that carry a fixed time-integrated energy per-area, and finding those that achieve the double requirement of maximizing the ionization that they induce, while having the shortest duration. We formulate this double-objective quantum optimal control problem by making use of the Pareto approach to multi-objective optimization, and the differential evolution genetic algorithm. The goal is to find out how a precise time-profiling of ultra-fast, large-bandwidth pulses may speed up the ionization process. We work on a simple one-dimensional model of hydrogen-like atoms (the Pöschl-Teller potential) that allows to tune the number of bound states that play a role in the ionization dynamics. We show how the detailed shape of the pulse accelerates the ionization, and how the presence or absence of bound states influences the velocity of the process.

  8. Ionized gas in the Irr galaxy IC 10: The emission spectrum and ionization sources

    NASA Astrophysics Data System (ADS)

    Arkhipova, V. P.; Egorov, O. V.; Lozinskaya, T. A.; Moiseev, A. V.

    2011-02-01

    We present the observations of the Irr galaxy IC 10 at the 6-m SAO telescope with the panoramic Multi-Pupil Fiber Spectrograph (MPFS). Based on the results of these observations and our long-slit spectroscopy performed previously, we have investigated the ionized-gas emission spectrum in the region of intense star formation and refined the gas metallicity estimates. We show that the “diagnostic diagrams” constructed from our observations agree best with the new improved ionization models by Martin-Manjon et al. Using these models, we have determined the electron density and gas ionization parameter and ionizing-cluster characteristics, the age and mass, from the spectra of the investigated HII regions. The cluster ages and masses are shown to be within the ranges 2.5-5 Myr and (0.2-1) × 105 M ⊗, respectively.

  9. Measurement of the first ionization potential of astatine by laser ionization spectroscopy

    PubMed Central

    Rothe, S.; Andreyev, A. N.; Antalic, S.; Borschevsky, A.; Capponi, L.; Cocolios, T. E.; De Witte, H.; Eliav, E.; Fedorov, D. V.; Fedosseev, V. N.; Fink, D. A.; Fritzsche, S.; Ghys, L.; Huyse, M.; Imai, N.; Kaldor, U.; Kudryavtsev, Yuri; Köster, U.; Lane, J. F. W.; Lassen, J.; Liberati, V.; Lynch, K. M.; Marsh, B. A.; Nishio, K.; Pauwels, D.; Pershina, V.; Popescu, L.; Procter, T. J.; Radulov, D.; Raeder, S.; Rajabali, M. M.; Rapisarda, E.; Rossel, R. E.; Sandhu, K.; Seliverstov, M. D.; Sjödin, A. M.; Van den Bergh, P.; Van Duppen, P.; Venhart, M.; Wakabayashi, Y.; Wendt, K. D. A.

    2013-01-01

    The radioactive element astatine exists only in trace amounts in nature. Its properties can therefore only be explored by study of the minute quantities of artificially produced isotopes or by performing theoretical calculations. One of the most important properties influencing the chemical behaviour is the energy required to remove one electron from the valence shell, referred to as the ionization potential. Here we use laser spectroscopy to probe the optical spectrum of astatine near the ionization threshold. The observed series of Rydberg states enabled the first determination of the ionization potential of the astatine atom, 9.31751(8) eV. New ab initio calculations are performed to support the experimental result. The measured value serves as a benchmark for quantum chemistry calculations of the properties of astatine as well as for the theoretical prediction of the ionization potential of superheavy element 117, the heaviest homologue of astatine. PMID:23673620

  10. Measurement of the first ionization potential of astatine by laser ionization spectroscopy

    NASA Astrophysics Data System (ADS)

    Rothe, S.; Andreyev, A. N.; Antalic, S.; Borschevsky, A.; Capponi, L.; Cocolios, T. E.; de Witte, H.; Eliav, E.; Fedorov, D. V.; Fedosseev, V. N.; Fink, D. A.; Fritzsche, S.; Ghys, L.; Huyse, M.; Imai, N.; Kaldor, U.; Kudryavtsev, Yuri; Köster, U.; Lane, J. F. W.; Lassen, J.; Liberati, V.; Lynch, K. M.; Marsh, B. A.; Nishio, K.; Pauwels, D.; Pershina, V.; Popescu, L.; Procter, T. J.; Radulov, D.; Raeder, S.; Rajabali, M. M.; Rapisarda, E.; Rossel, R. E.; Sandhu, K.; Seliverstov, M. D.; Sjödin, A. M.; van den Bergh, P.; van Duppen, P.; Venhart, M.; Wakabayashi, Y.; Wendt, K. D. A.

    2013-05-01

    The radioactive element astatine exists only in trace amounts in nature. Its properties can therefore only be explored by study of the minute quantities of artificially produced isotopes or by performing theoretical calculations. One of the most important properties influencing the chemical behaviour is the energy required to remove one electron from the valence shell, referred to as the ionization potential. Here we use laser spectroscopy to probe the optical spectrum of astatine near the ionization threshold. The observed series of Rydberg states enabled the first determination of the ionization potential of the astatine atom, 9.31751(8) eV. New ab initio calculations are performed to support the experimental result. The measured value serves as a benchmark for quantum chemistry calculations of the properties of astatine as well as for the theoretical prediction of the ionization potential of superheavy element 117, the heaviest homologue of astatine.

  11. Measurement of the first ionization potential of astatine by laser ionization spectroscopy.

    PubMed

    Rothe, S; Andreyev, A N; Antalic, S; Borschevsky, A; Capponi, L; Cocolios, T E; De Witte, H; Eliav, E; Fedorov, D V; Fedosseev, V N; Fink, D A; Fritzsche, S; Ghys, L; Huyse, M; Imai, N; Kaldor, U; Kudryavtsev, Yuri; Köster, U; Lane, J F W; Lassen, J; Liberati, V; Lynch, K M; Marsh, B A; Nishio, K; Pauwels, D; Pershina, V; Popescu, L; Procter, T J; Radulov, D; Raeder, S; Rajabali, M M; Rapisarda, E; Rossel, R E; Sandhu, K; Seliverstov, M D; Sjödin, A M; Van den Bergh, P; Van Duppen, P; Venhart, M; Wakabayashi, Y; Wendt, K D A

    2013-01-01

    The radioactive element astatine exists only in trace amounts in nature. Its properties can therefore only be explored by study of the minute quantities of artificially produced isotopes or by performing theoretical calculations. One of the most important properties influencing the chemical behaviour is the energy required to remove one electron from the valence shell, referred to as the ionization potential. Here we use laser spectroscopy to probe the optical spectrum of astatine near the ionization threshold. The observed series of Rydberg states enabled the first determination of the ionization potential of the astatine atom, 9.31751(8) eV. New ab initio calculations are performed to support the experimental result. The measured value serves as a benchmark for quantum chemistry calculations of the properties of astatine as well as for the theoretical prediction of the ionization potential of superheavy element 117, the heaviest homologue of astatine.

  12. First successful ionization of Lr (Z = 103) by a surface-ionization technique

    SciTech Connect

    Sato, Tetsuya K. Sato, Nozomi; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Ooe, Kazuhiro; Miyashita, Sunao; Schädel, Matthias; Kaneya, Yusuke; Nagame, Yuichiro; Osa, Akihiko; Ichikawa, Shin-ichi; Stora, Thierry; Kratz, Jens Volker

    2013-02-15

    We have developed a surface ionization ion-source as part of the JAEA-ISOL (Isotope Separator On-Line) setup, which is coupled to a He/CdI{sub 2} gas-jet transport system to determine the first ionization potential of the heaviest actinide lawrencium (Lr, Z = 103). The new ion-source is an improved version of the previous source that provided good ionization efficiencies for lanthanides. An additional filament was newly installed to give better control over its operation. We report, here, on the development of the new gas-jet coupled surface ion-source and on the first successful ionization and mass separation of 27-s {sup 256}Lr produced in the {sup 249}Cf + {sup 11}B reaction.

  13. First successful ionization of Lr (Z = 103) by a surface-ionization technique.

    PubMed

    Sato, Tetsuya K; Sato, Nozomi; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Ooe, Kazuhiro; Miyashita, Sunao; Schädel, Matthias; Kaneya, Yusuke; Nagame, Yuichiro; Osa, Akihiko; Ichikawa, Shin-ichi; Stora, Thierry; Kratz, Jens Volker

    2013-02-01

    We have developed a surface ionization ion-source as part of the JAEA-ISOL (Isotope Separator On-Line) setup, which is coupled to a He/CdI2 gas-jet transport system to determine the first ionization potential of the heaviest actinide lawrencium (Lr, Z = 103). The new ion-source is an improved version of the previous source that provided good ionization efficiencies for lanthanides. An additional filament was newly installed to give better control over its operation. We report, here, on the development of the new gas-jet coupled surface ion-source and on the first successful ionization and mass separation of 27-s (256)Lr produced in the (249)Cf + (11)B reaction.

  14. First successful ionization of Lr (Z = 103) by a surface-ionization technique

    NASA Astrophysics Data System (ADS)

    Sato, Tetsuya K.; Sato, Nozomi; Asai, Masato; Tsukada, Kazuaki; Toyoshima, Atsushi; Ooe, Kazuhiro; Miyashita, Sunao; Schädel, Matthias; Kaneya, Yusuke; Nagame, Yuichiro; Osa, Akihiko; Ichikawa, Shin-ichi; Stora, Thierry; Kratz, Jens Volker

    2013-02-01

    We have developed a surface ionization ion-source as part of the JAEA-ISOL (Isotope Separator On-Line) setup, which is coupled to a He/CdI2 gas-jet transport system to determine the first ionization potential of the heaviest actinide lawrencium (Lr, Z = 103). The new ion-source is an improved version of the previous source that provided good ionization efficiencies for lanthanides. An additional filament was newly installed to give better control over its operation. We report, here, on the development of the new gas-jet coupled surface ion-source and on the first successful ionization and mass separation of 27-s 256Lr produced in the 249Cf + 11B reaction.

  15. Determination of the first ionization potential of berkelium and californium by resonance ionization mass spectroscopy

    SciTech Connect

    Nunnemann, M.; Eberhardt, K.; Erdmann, N.; Herrmann, G.; Huber, G.; Koehler, S.; Kratz, J. V.; Naehler, A.; Passler, G.; Trautmann, N.

    1997-01-15

    Resonance ionization mass spectroscopy (RIMS) is used for the precise determination of the first ionization potential (IP) of transuranium elements. Small amounts of material ({approx_equal}0.4 ng) are sufficient for these measurements due to the high sensitivity of RIMS enabling the investigation of the actinides beyond plutonium, which are accessible only in limited amounts and difficult to handle due to their high radioactivity. The method presented takes advantage of the dependence of the ionization threshold on an external static electric field. With samples of 10{sup 12} atoms of {sup 249}Bk and {sup 249}Cf experimental values for the first ionization potentials of IP{sub Bk}=49989(2) cm{sup -1} and IP{sub Cf}=50665(2) cm{sup -1} were obtained.

  16. Determination of the first ionization potential of berkelium and californium by resonance ionization mass spectroscopy

    SciTech Connect

    Nunnemann, M.; Eberhardt, K.; Erdmann, N.; Herrmann, G.; Huber, G.; Koehler, S.; Kratz, J.V.; Naehler, A.; Passler, G.; Trautmann, N.

    1997-01-01

    Resonance ionization mass spectroscopy (RIMS) is used for the precise determination of the first ionization potential ({ital IP}) of transuranium elements. Small amounts of material ({approx}0.4ng) are sufficient for these measurements due to the high sensitivity of RIMS enabling the investigation of the actinides beyond plutonium, which are accessible only in limited amounts and difficult to handle due to their high radioactivity. The method presented takes advantage of the dependence of the ionization threshold on an external static electric field. With samples of 10{sup 12} atoms of {sup 249}Bk and {sup 249}Cf experimental values for the first ionization potentials of IP{sub Bk}=49989(2)cm{sup {minus}1} and IP{sub Cf}=50665(2)cm{sup {minus}1} were obtained. {copyright} {ital 1997 American Institute of Physics.}

  17. Amplitude distribution of ionization jerks in ionization-chamber ASK-1 according long-term measurements

    NASA Astrophysics Data System (ADS)

    Timofeev, Vladislav

    2016-07-01

    As part of the Yakut complex systems by measuring the intensity of cosmic rays has a unique device spherical - ionization chamber ASK-1 with a lead screen thickness of 12 cm. The camera allows you to explore the physical characteristics of the so-called "ionization jerks " - sharp increases ionization current caused by the passage through the device much ionizing particles of cosmic origin. Due to a large increase in current nuclear cascade "showers", formed mainly by particles of cosmic rays in the camera screen. Over the entire period of observation (50 years old) camera ASK-1 was registered 59125 aftershocks. Their nature and properties still does not sufficiently studied, especially in medium and large amplitudes.

  18. Ground Levels and Ionization Energies for the Neutral Atoms

    National Institute of Standards and Technology Data Gateway

    SRD 111 Ground Levels and Ionization Energies for the Neutral Atoms (Web, free access)   Data for ground state electron configurations and ionization energies for the neutral atoms (Z = 1-104) including references.

  19. STABILIZATION OF EEE VIRUS AGAINST ULTRAVIOLET AND IONIZING RADIATIONS

    DTIC Science & Technology

    inactivation were effective as well against ionizing radiation. However, known radioprotective compounds, such as cysteamine , which also protected EEE virus against ionizing radiation, were completely ineffective against UV radiation.

  20. Picosecond ionization dynamics in femtosecond filaments at high pressures

    NASA Astrophysics Data System (ADS)

    Gao, Xiaohui; Patwardhan, Gauri; Schrauth, Samuel; Zhu, Daiwei; Popmintchev, Tenio; Kapteyn, Henry C.; Murnane, Margaret M.; Romanov, Dmitri A.; Levis, Robert J.; Gaeta, Alexander L.

    2017-01-01

    We investigate the plasma dynamics inside a femtosecond-pulse-induced filament generated in an argon gas for a wide range of pressures up to 60 bar. At higher pressures, we observe ionization immediately following a pulse, with up to a threefold increase in the electron density within 30 ps after the filamentary propagation of a femtosecond pulse. Our study suggests that this picosecond evolution can be attributed to collisional ionization including Penning and associative ionizations and electron-impact ionization of excited atoms generated during the pulse. The dominance of excited atoms over ionized atoms at the end of the pulse also indicates an intrapulse inhibition of avalanche ionization. This delayed ionization dynamics provides evidence for diagnosing atomic and molecular excitation and ionization in intense laser interaction with high-pressure gases.

  1. IONIZATION IN ATMOSPHERES OF BROWN DWARFS AND EXTRASOLAR PLANETS. II. DUST-INDUCED COLLISIONAL IONIZATION

    SciTech Connect

    Helling, Ch.; Jardine, M.; Mokler, F.

    2011-08-10

    Observations have shown that continuous radio emission and also sporadic H{alpha} and X-ray emission are prominent in singular, low-mass objects later than spectral class M. These activity signatures are interpreted as being caused by coupling of an ionized atmosphere to the stellar magnetic field. What remains a puzzle, however, is the mechanism by which such a cool atmosphere can produce the necessary level of ionization. At these low temperatures, thermal gas processes are insufficient, but the formation of clouds sets in. Cloud particles can act as seeds for electron avalanches in streamers that ionize the ambient gas, and can lead to lightning and indirectly to magnetic field coupling, a combination of processes also expected for protoplanetary disks. However, the precondition is that the cloud particles are charged. We use results from DRIFT-PHOENIX model atmospheres to investigate collisional processes that can lead to the ionization of dust grains inside clouds. We show that ionization by turbulence-induced dust-dust collisions is the most efficient kinetic process. The efficiency is highest in the inner cloud where particles grow quickly and, hence, the dust-to-gas ratio is high. Dust-dust collisions alone are not sufficient to improve the magnetic coupling of the atmosphere inside the cloud layers, but the charges supplied either on grains or within the gas phase as separated electrons can trigger secondary nonlinear processes. Cosmic rays are likely to increase the global level of ionization, but their influence decreases if a strong, large-scale magnetic field is present as on brown dwarfs. We suggest that although thermal gas ionization declines in objects across the fully convective boundary, dust charging by collisional processes can play an important role in the lowest mass objects. The onset of atmospheric dust may therefore correlate with the anomalous X-ray and radio emission in atmospheres that are cool, but charged more than expected by pure

  2. Electron Impact Ionization and Dissociative Ionization of C2H2

    NASA Technical Reports Server (NTRS)

    Srivastava, S. K.

    1995-01-01

    By utilizing a crossed electron beam collision geometry, a combination of time-of-flight (TOF) and quadrupole mass spectrometers, and the relative flow technique1 normalized values of cross sections and appearance energies (AP) were obtained for the formation of singly and multiply ionized species resulting from the ionization and dissociation of C2H2. Details ont he apparatus and technique have been published previously.2,3.

  3. Theoretical study of electron impact-ionization of molecules

    NASA Astrophysics Data System (ADS)

    Al-Hagan, Ola

    There has been impressive progress in the area of theoretical treatments of electron impact ionization (e,2e) of atoms and molecules in the last decade. Most recently, low to intermediate incident electron energies have been reported for molecular systems. In this dissertation, different theoretical models will be used to calculate the fully differential cross section (FDCS) for (e,2e) processes for low to intermediate incident electron energies for a variety of final state electron angles and energies for the diatomic molecules H2 and N2, the triatomic molecule H2O, and the boimolecule HCOOH. In addition, there has been a large amount of interest in diatomic molecules inspired by the possibility of observing an interference effect due to the two molecular centers playing the role of a double slit. In this dissertation, the interference effect for the diatomic molecules H2 and N2 will be examined. Finally, there is presently considerable experimental effort directed towards measuring the FDCS for a specific molecular orientation. Most recently, the FDCS for single ionization of aligned hydrogen molecules was measured by Alexander Dorn's experimental group in Heidelberg, Germany. These measurements were successful for the first time to observe features of the FDCS for different alignment of H2. Theoretical calculations for aligned H2 will be presented. These calculations were able to obtain good agreement with the experimental data especially in the binary peak region.

  4. Ionization damage in NPN transistors caused by lower energy electrons

    NASA Astrophysics Data System (ADS)

    Li, Xingji; Xiao, Jingdong; Liu, Chaoming; Zhao, Zhiming; Geng, Hongbin; Lan, Mujie; Yang, Dezhuang; He, Shiyu

    2010-09-01

    Electrical degradation of two type NPN bipolar junction transistors (BJTs) with different emitter sizes was examined under exposures of 70 and 110 keV electrons. Base and collector currents as a function of base-emitter voltage were in-situ measured during exposure. Experimental results show that both the 70 and 110 keV electrons produce an evident ionization damage to the NPN BJTs. With increasing fluence, collector currents of the NPN BJTs hardly change in the whole range of base-emitter voltage from 0 to 1.2 V, while base currents increase in a gradually mitigative trend. Base currents vary more at lower base-emitter voltages than at higher ones for a given fluence. The change in the reciprocal of current gain at a fixed base-emitter voltage of 0.65 V increases non-linearly at lower fluences and tends to be gradually saturated at higher fluences. Sensitivity to ionization damage increases for BJTs with an emitter having a larger perimeter-to-area ratio.

  5. MOLECULAR AND IONIZED HYDROGEN IN 30 DORADUS. I. IMAGING OBSERVATIONS

    SciTech Connect

    Yeh, Sherry C. C.; Seaquist, Ernest R.; Matzner, Christopher D.; Pellegrini, Eric W.

    2015-07-10

    We present the first fully calibrated H{sub 2} 1–0 S(1) image of the entire 30 Doradus nebula. The observations were conducted using the NOAO Extremely Wide-field Infrared Imager (NEWFIRM) on the CTIO 4 m Blanco Telescope. Together with a NEWFIRM Brγ image of 30 Doradus, our data reveal the morphologies of the warm molecular gas and ionized gas in 30 Doradus. The brightest H{sub 2}-emitting area, which extends from the northeast to the southwest of R136, is a photodissociation region (PDR) viewed face-on, while many clumps and pillar features located at the outer shells of 30 Doradus are PDRs viewed edge-on. Based on the morphologies of H{sub 2}, Brγ, CO, and 8 μm emission, the H{sub 2} to Brγ line ratio, and Cloudy models, we find that the H{sub 2} emission is formed inside the PDRs of 30 Doradus, 2–3 pc to the ionization front of the H ii region, in a relatively low-density environment <10{sup 4} cm{sup −3}. Comparisons with Brγ, 8 μm, and CO emission indicate that H{sub 2} emission is due to fluorescence, and provide no evidence for shock excited emission of this line.

  6. Two-Color Laser Resonance Ionization Spectroscopy of Zirconium Atoms

    NASA Astrophysics Data System (ADS)

    Hasegawa, Shuichi; Nagamoto, Daisuke

    2017-10-01

    We have performed two-color laser resonance ionization spectroscopy of zirconium atoms to measure the energies of excited states below the third ionization limit. The number of intermediate states that we observed is 19, and energies deduced from the experiments agree with previous data. Complex ionization spectra of the excited states were observed through the intermediate states. The values of the first, second, and third ionization limits were derived from the Rydberg series of the spectra with quantum defect theory.

  7. High-efficiency electron ionizer for a mass spectrometer array

    NASA Technical Reports Server (NTRS)

    Chutjian, Ara (Inventor); Darrach, Murray R. (Inventor); Orient, Otto J. (Inventor)

    2001-01-01

    The present invention provides an improved electron ionizer for use in a quadrupole mass spectrometer. The improved electron ionizer includes a repeller plate that ejects sample atoms or molecules, an ionizer chamber, a cathode that emits an electron beam into the ionizer chamber, an exit opening for excess electrons to escape, at least one shim plate to collimate said electron beam, extraction apertures, and a plurality of lens elements for focusing the extracted ions onto entrance apertures.

  8. A nanoscale soft-ionization membrane: A novel ionizer for ion mobility spectrometers for space applications

    NASA Astrophysics Data System (ADS)

    Hartley, Frank T.; Kanik, Isik

    2002-11-01

    The Jet Propulsion Laboratory (JPL) has developed a novel nanometer-thick "Soft Ionization Membrane" (SIM) which is capable of ionizing nearly 100% of the gases that pass through it. Both sides of the membrane are coated with a metallic conducting film. A modest potential of less than 10 Volts across the membrane produces an electric field in excess of 107 V/cm over a region that is smaller than the mean free path of gas molecules which ionizes the neutral molecules that passing through. Because the region of high electric field is smaller than the mean free path of gas molecules, there are virtually no high energy collisions and the system does not suffer from the fatal problem of avalanche breakdown. The soft ionization mechanism does not fracture the medium or cause any secondary ionization. Thus, a truly new ionization technique is enabled by a simple nanoscale micromachined device. The SIM is tiny, rugged and well suited for a wide variety of applications ranging from space micropropulsion systems to miniature analytical separation devices. In this paper we focus our attention on ion mobility spectrometers (IMSs) as a potential candidate to be incorporated with SIM.

  9. Atmospheric Pressure Ionization Using a High Voltage Target Compared to Electrospray Ionization

    NASA Astrophysics Data System (ADS)

    Lubin, Arnaud; Bajic, Steve; Cabooter, Deirdre; Augustijns, Patrick; Cuyckens, Filip

    2017-02-01

    A new atmospheric pressure ionization (API) source, viz. UniSpray, was evaluated for mass spectrometry (MS) analysis of pharmaceutical compounds by head-to-head comparison with electrospray ionization (ESI) on the same high-resolution MS system. The atmospheric pressure ionization source is composed of a grounded nebulizer spraying onto a high voltage, cylindrical stainless steel target. Molecules are ionized in a similar fashion to electrospray ionization, predominantly producing protonated or deprotonated species. Adduct formation (e.g., proton and sodium adducts) and in-source fragmentation is shown to be almost identical between the two sources. The performance of the new API source was compared with electrospray by infusion of a mix of 22 pharmaceutical compounds with a wide variety of functional groups and physico-chemical properties (molecular weight, logP, and pKa) in more than 100 different conditions (mobile phase strength, solvents, pH, and flow rate). The new API source shows an intensity gain of a factor 2.2 compared with ESI considering all conditions on all compounds tested. Finally, some hypotheses on the ionization mechanism, similarities, and differences with ESI, are discussed.

  10. A mechanism for ionization of nonvolatile compounds in mass spectrometry: considerations from MALDI and inlet ionization.

    PubMed

    Trimpin, Sarah; Wang, Beixi; Inutan, Ellen D; Li, Jing; Lietz, Christopher B; Harron, Andrew; Pagnotti, Vincent S; Sardelis, Diana; McEwen, Charles N

    2012-10-01

    Mechanistic arguments relative to matrix-assisted laser desorption/ionization (MALDI) mass spectrometry (MS) address observations that predominately singly charged ions are detected. However, recently a matrix assisted laser ablation method, laserspray ionization (LSI), was introduced that can use the same sample preparation and laser as MALDI, but produce highly charged ions from proteins. In MALDI, ions are generated from neutral molecules by the photon energy provided to a matrix, while in LSI ions are produced inside a heated inlet tube linking atmospheric pressure and the first vacuum region of the mass spectrometer. Some LSI matrices also produce highly charged ions with MALDI ion sources operated at intermediate pressure or high vacuum. The operational similarity of LSI to MALDI, and the large difference in charge states observed by these methods, provides information of fundamental importance to proposed ionization mechanisms for LSI and MALDI. Here, we present data suggesting that the prompt and delayed ionization reported for vacuum MALDI are both fast processes relative to producing highly charged ions by LSI. The energy supplied to produce these charged clusters/droplets as well as their size and time available for desolvation are determining factors in the charge states of the ions observed. Further, charged droplets/clusters may be a common link for ionization of nonvolatile compounds by a variety of MS ionization methods, including MALDI and LSI.

  11. Graphene coated silica applied for high ionization matrix assisted laser desorption/ionization mass spectrometry: A novel approach for environmental and biomolecule analysis.

    PubMed

    Nasser Abdelhamid, Hani; Wu, Bo-Sgum; Wu, Hui-Fen

    2014-08-01

    The integration of nanotechnology with mass spectrometry for sensitive and selective detection of molecules is a hot/important field of research. Synthesis of graphene (G) coated with mesoporous silica (SiO2, G@SiO2) for mass spectrometric application has been demonstrated. For the first time, we proposed the significant role of surfactant that used during the synthesis of mesorporous silicate (SiO2) in mass spectrometry. It was noticed that G could initiate SiO2 via surfactants which work as initiators for further ionization. The porosity of SiO2 trapped the analytes that was released and ionized with the surfactant fragments. Undoubtedly, strong background interferences were present in the case of organic matrix, which greatly obscured the detection of low molecular weight compounds. G@SiO2 nanocomposite affords several advantages, such as the ability to detect small molecules (<500Da), high sample localization through silica mesoporosity, and high ionization efficiency over than G or conventional matrices. The high performance of G@SiO2 is not only due to the large surface area but also due to high desorption/ionization efficiency of inevitably surfactant (cetyltrimethylammonium chloride, CATB). Unlike the conventional MALDI-MS, the G@SiO2-MS is capable of generating multiply charged polysaccharides. The present method was validated to detect surfactants with low limits of detection.

  12. Importance of electric fields from ionized nanoparticles for radiation therapy

    NASA Astrophysics Data System (ADS)

    Shmatov, M. L.

    2017-05-01

    A model is presented in which electric fields from ionized particles in a biological tissue enhance the biological effect of ionizing radiation. The model is based on the data on enhancing the gamma radiation effect on biological cells by static electric fields and on estimates of the typical intensities of electric fields from ionized nanoparticles in a biological tissue.

  13. Method and apparatus to monitor a beam of ionizing radiation

    DOEpatents

    Blackburn, Brandon W.; Chichester, David L.; Watson, Scott M.; Johnson, James T.; Kinlaw, Mathew T.

    2015-06-02

    Methods and apparatus to capture images of fluorescence generated by ionizing radiation and determine a position of a beam of ionizing radiation generating the fluorescence from the captured images. In one embodiment, the fluorescence is the result of ionization and recombination of nitrogen in air.

  14. A numerical scheme for ionizing shock waves

    SciTech Connect

    Aslan, Necdet . E-mail: naslan@yeditepe.edu.tr; Mond, Michael

    2005-12-10

    A two-dimensional (2D) visual computer code to solve the steady state (SS) or transient shock problems including partially ionizing plasma is presented. Since the flows considered are hypersonic and the resulting temperatures are high, the plasma is partially ionized. Hence the plasma constituents are electrons, ions and neutral atoms. It is assumed that all the above species are in thermal equilibrium, namely, that they all have the same temperature. The ionization degree is calculated from Saha equation as a function of electron density and pressure by means of a nonlinear Newton type root finding algorithms. The code utilizes a wave model and numerical fluctuation distribution (FD) scheme that runs on structured or unstructured triangular meshes. This scheme is based on evaluating the mesh averaged fluctuations arising from a number of waves and distributing them to the nodes of these meshes in an upwind manner. The physical properties (directions, strengths, etc.) of these wave patterns are obtained by a new wave model: ION-A developed from the eigen-system of the flux Jacobian matrices. Since the equation of state (EOS) which is used to close up the conservation laws includes electronic effects, it is a nonlinear function and it must be inverted by iterations to determine the ionization degree as a function of density and temperature. For the time advancement, the scheme utilizes a multi-stage Runge-Kutta (RK) algorithm with time steps carefully evaluated from the maximum possible propagation speed in the solution domain. The code runs interactively with the user and allows to create different meshes to use different initial and boundary conditions and to see changes of desired physical quantities in the form of color and vector graphics. The details of the visual properties of the code has been published before (see [N. Aslan, A visual fluctuation splitting scheme for magneto-hydrodynamics with a new sonic fix and Euler limit, J. Comput. Phys. 197 (2004) 1

  15. An instrument combining an electrospray ionization source and a velocity-map imaging spectrometer for studying delayed electron emission of polyanions

    NASA Astrophysics Data System (ADS)

    Concina, Bruno; Papalazarou, Evangelos; Barbaire, Marc; Clavier, Christian; Maurelli, Jacques; Lépine, Franck; Bordas, Christian

    2016-03-01

    An instrument combining an electrospray ionization source and a velocity-map imaging (VMI) spectrometer has been developed in order to study the delayed electron emission of molecular anions and especially of polyanions. It operates at a high repetition rate (kHz) in order to increase the acquisition speed. The VMI spectrometer has been upgraded for nanosecond time resolution by gating the voltages applied on the position-sensitive detector. Kinetic energy release distribution of thermionic emission (without any contribution from direct detachment) can be recorded for well-defined delays after the nanosecond laser excitation. The capability of the instrument is demonstrated by recording photodetachment spectra of the benchmark C60- anion and C842- dianion.

  16. An instrument combining an electrospray ionization source and a velocity-map imaging spectrometer for studying delayed electron emission of polyanions

    SciTech Connect

    Concina, Bruno Papalazarou, Evangelos; Barbaire, Marc; Clavier, Christian; Maurelli, Jacques; Lépine, Franck; Bordas, Christian

    2016-03-15

    An instrument combining an electrospray ionization source and a velocity-map imaging (VMI) spectrometer has been developed in order to study the delayed electron emission of molecular anions and especially of polyanions. It operates at a high repetition rate (kHz) in order to increase the acquisition speed. The VMI spectrometer has been upgraded for nanosecond time resolution by gating the voltages applied on the position-sensitive detector. Kinetic energy release distribution of thermionic emission (without any contribution from direct detachment) can be recorded for well-defined delays after the nanosecond laser excitation. The capability of the instrument is demonstrated by recording photodetachment spectra of the benchmark C{sub 60}{sup −} anion and C{sub 84}{sup 2−} dianion.

  17. Intravenous correction of neonatal hypomagnesemia: effect on ionized magnesium.

    PubMed

    Maggioni, A; Orzalesi, M; Mimouni, F B

    1998-04-01

    Neonatal hypomagnesemia is defined as total magnesium (TMg) < or = 0.65 mmol/L (1.6 mg/dl). However, magnesium (Mg) deficiency and sufficiency overlap at serum values of 0.57 to 0.74 mmol/L (1.4 to 1.8 mg/dl). We hypothesized that (1) some infants with TMg < or = 0.65 mmol/L (1.6 mg/dl) have normal ionized Mg values (normal neonatal range 0.40 to 0.56 mmol/L (0.97 to 1.36 mg/dl)); (2) the dose (6.0 mg of elemental Mg/kg) used to correct hypomagnesemia does not lead to elevation of ionized Mg; (3) after intravenous magnesium sulfate infusion, ionized calcium increases in patients with low baseline ionized Mg and decreases in patients with normal baseline ionized Mg. We recruited 22 neonates with TMg < or = 1.6 mg/dl. They received intravenous sulfate (6 mg elemental Mg/kg) over a 1-hour period. Serum TMg, ionized Mg, and ionized Ca were measured before and after magnesium sulfate infusion. An ion-selective electrode was used to allow direct measurement of ionized Mg and ionized Ca. Thirteen (59%) of 22 neonates with TMg < or = 0.65 mmol/L (1.6 mg/dl) had normal IMg. In 7 (31%) of 22 cases ionized Mg increased slightly above 0.56 mmol/L (1.36 mg/dl); the maximum value was 0.61 mmol/L (1.48 mg/dl). The change in ionized Ca concentrations and the baseline ionized Mg value were inversely correlated (r = -0.79; p < 0.0001). (1) Measurement of ionized Mg should prevent overdiagnosis and treatment of hypomagnesemia. (2) The dose used in this study is safe. (3) Ionized Mg concentrations are inversely correlated to the response of ionized Ca concentrations to an Mg load.

  18. HCO(+) ionization from SGR1806-20

    NASA Technical Reports Server (NTRS)

    Hannikainen, D.; Durouchoux, P.; Vilhu, O.; Huovelin, J.; Corbel, S.; Wallyn, P.

    1997-01-01

    The region surrounding the soft gamma ray repeater SGR 1806-20 in the HCO(+) (J = 1-0) transition was observed. Previous observations of compact Galactic objects suggest that a link exists between these objects and molecular clouds in which they are possibly embedded. Such a link would help explain some of the phenomena observed from these objects. A measure of the ionization rate as a function of distance from the source implies that the cloud is associated with the source. The abundance of HCO(+), which varies with increasing or decreasing ionization rates, is considered to be an ideal tool for this measurement. The observations acquired in the direction of the nebula surrounding SGR 1806-20 are presented, and the resulting 7 x 12 arcmin map derived from the HCO(+) data is shown.

  19. Atmospheric Ionizing Radiation and Human Exposure

    NASA Technical Reports Server (NTRS)

    Wilson, John W.; Mertens, Christopher J.; Goldhagen, Paul; Friedberg, W.; DeAngelis, G.; Clem, J. M.; Copeland, K.; Bidasaria, H. B.

    2005-01-01

    Atmospheric ionizing radiation is of interest, apart from its main concern of aircraft exposures, because it is a principal source of human exposure to radiations with high linear energy transfer (LET). The ionizing radiations of the lower atmosphere near the Earth s surface tend to be dominated by the terrestrial radioisotopes. especially along the coastal plain and interior low lands, and have only minor contributions from neutrons (11 percent). The world average is substantially larger but the high altitude cities especially have substantial contributions from neutrons (25 to 45 percent). Understanding the world distribution of neutron exposures requires an improved understanding of the latitudinal, longitudinal, altitude and spectral distribution that depends on local terrain and time. These issues are being investigated in a combined experimental and theoretical program. This paper will give an overview of human exposures and describe the development of improved environmental models.

  20. Atmospheric Ionizing Radiation and Human Exposure

    NASA Technical Reports Server (NTRS)

    Wilson, J. W.; Goldhagen, P.; Friedberg, W.; DeAngelis, G.; Clem, J. M.; Copeland, K.; Bidasaria, H. B.

    2004-01-01

    Atmospheric ionizing radiation is of interest, apart from its main concern of aircraft exposures, because it is a principal source of human exposure to radiations with high linear energy transfer (LET). The ionizing radiations of the lower atmosphere near the Earth s surface tend to be dominated by the terrestrial radioisotopes especially along the coastal plain and interior low lands and have only minor contributions from neutrons (11 percent). The world average is substantially larger but the high altitude cities especially have substantial contributions from neutrons (25 to 45 percent). Understanding the world distribution of neutron exposures requires an improved understanding of the latitudinal, longitudinal, altitude and spectral distribution that depends on local terrain and time. These issues are being investigated in a combined experimental and theoretical program. This paper will give an overview of human exposures and describe the development of improved environmental models.