Sample records for atomic nuclei issue

  1. Atomic Mass and Nuclear Binding Energy for U-287 (Uranium)

    NASA Astrophysics Data System (ADS)

    Sukhoruchkin, S. I.; Soroko, Z. N.

    This document is part of the Supplement containing the complete sets of data of Subvolume B `Nuclei with Z = 55 - 100' of Volume 22 `Nuclear Binding Energies and Atomic Masses' of Landolt-Börnstein - Group I `Elementary Particles, Nuclei and Atoms', and additionally including data for nuclei with Z = 101 - 130. It provides atomic mass, mass excess, nuclear binding energy, nucleon separation energies, Q-values, and nucleon residual interaction parameters for atomic nuclei of the isotope U-287 (Uranium, atomic number Z = 92, mass number A = 287).

  2. Atomic Mass and Nuclear Binding Energy for Ac-212 (Actinium)

    NASA Astrophysics Data System (ADS)

    Sukhoruchkin, S. I.; Soroko, Z. N.

    This document is part of the Supplement containing the complete sets of data of Subvolume B `Nuclei with Z = 55 - 100' of Volume 22 `Nuclear Binding Energies and Atomic Masses' of Landolt-Börnstein - Group I `Elementary Particles, Nuclei and Atoms', and additionally including data for nuclei with Z = 101 - 130. It provides atomic mass, mass excess, nuclear binding energy, nucleon separation energies, Q-values, and nucleon residual interaction parameters for atomic nuclei of the isotope Ac-212 (Actinium, atomic number Z = 89, mass number A = 212).

  3. Atomic Mass and Nuclear Binding Energy for I-131 (Iodine)

    NASA Astrophysics Data System (ADS)

    Sukhoruchkin, S. I.; Soroko, Z. N.

    This document is part of the Supplement containing the complete sets of data of Subvolume A `Nuclei with Z = 1 - 54' of Volume 22 `Nuclear Binding Energies and Atomic Masses' of Landolt-Börnstein - Group I `Elementary Particles, Nuclei and Atoms'. It provides atomic mass, mass excess, nuclear binding energy, nucleon separation energies, Q-values, and nucleon residual interaction parameters for atomic nuclei of the isotope I-131 (Iodine, atomic number Z = 53, mass number A = 131).

  4. Atomic Mass and Nuclear Binding Energy for F-22 (Fluorine)

    NASA Astrophysics Data System (ADS)

    Sukhoruchkin, S. I.; Soroko, Z. N.

    This document is part of the Supplement containing the complete sets of data of Subvolume A `Nuclei with Z = 1 - 54' of Volume 22 `Nuclear Binding Energies and Atomic Masses' of Landolt-Börnstein - Group I `Elementary Particles, Nuclei and Atoms'. It provides atomic mass, mass excess, nuclear binding energy, nucleon separation energies, Q-values, and nucleon residual interaction parameters for atomic nuclei of the isotope F-22 (Fluorine, atomic number Z = 9, mass number A = 22).

  5. Energy levels for Ac-212 (Actinium-212)

    NASA Astrophysics Data System (ADS)

    Sukhoruchkin, S. I.; Soroko, Z. N.

    This document is part of Subvolume C `Tables of Excitations of Proton- and Neutron-rich Unstable Nuclei' of Volume 19 `Nuclear States from Charged Particle Reactions' of Landolt-Börnstein - Group I `Elementary Particles, Nuclei and Atoms'. It provides energy levels for atomic nuclei of the isotope Ac-212 (actinium, atomic number Z = 89, mass number A = 212).

  6. Recent trends in precision measurements of atomic and nuclear properties with lasers and ion traps

    NASA Astrophysics Data System (ADS)

    Block, Michael

    2017-11-01

    The X. international workshop on "Application of Lasers and Storage Devices in Atomic Nuclei Research" took place in Poznan in May 2016. It addressed the latest experimental and theoretical achievements in laser and ion trap-based investigations of radionuclides, highly charged ions and antiprotons. The precise determination of atomic and nuclear properties provides a stringent benchmark for theoretical models and eventually leads to a better understanding of the underlying fundamental interactions and symmetries. This article addresses some general trends in this field and highlights select recent achievements presented at the workshop. Many of these are covered in more detail within the individual contributions to this special issue of Hyperfine Interactions.

  7. Effect of local structures on crystallization in deeply undercooled metallic glass-forming liquids

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Jiang, S. Q.; Li, M. Z., E-mail: maozhili@ruc.edu.cn; Wu, Z. W.

    2016-04-21

    The crystallization mechanism in deeply undercooled ZrCu metallic glass-forming liquids was investigated via molecular dynamics simulations. It was found that the crystallization process is mainly controlled by the growth of crystal nuclei formed by the BCC-like atomic clusters, consistent with experimental speculations. The crystallization rate is found to relate to the number of growing crystal nuclei in the crystallization process. The crystallization rate in systems with more crystal nuclei is significantly hindered by the larger surface fractions of crystal nuclei and their different crystalline orientations. It is further revealed that in the crystallization in deeply undercooled regions, the BCC-like crystalmore » nuclei are formed from the inside of the precursors formed by the FCC-like atomic clusters, and growing at the expense of the precursors. Meanwhile, the precursors are expanding at the expense of the outside atomic clusters. This process is consistent with the so-called Ostwald step rule. The atomic structures of metallic glasses are found to have significant impact on the subsequent crystallization process. In the Zr{sub 85}Cu{sub 15} system, the stronger spatial correlation of Cu atoms could hinder the crystallization processes in deeply undercooled regions.« less

  8. Understanding glass-forming ability through sluggish crystallization of atomically thin metallic glassy films

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Sun, Y. T.; Cao, C. R.; Huang, K. Q.

    2014-08-04

    The glass-forming ability (GFA) of an alloy, closely related to its ability to resist crystallization, is a crucial issue in condensed matter physics. So far, the studies on GFA are mostly statistical and empirical guides. Benefiting from the ultrahigh thermal stability of ultrathin metallic glassy film and high resolution spherical aberration-corrected transmission electron microscope, the crystallization of atomically thin ZrCu and its microalloyed ZrCuAl glasses with markedly different GFA was investigated at the atomic scale. We find the Zr diffusivity estimated from the density of nuclei is dramatically decreased by adding of Al, which is the major reason for themore » much better GFA of the ZrCuAl metallic glass.« less

  9. Research with Radioactive Targets

    NASA Astrophysics Data System (ADS)

    Ahle, Larry

    2004-10-01

    Obtaining precise information about neutron capture cross-sections for s-process branch points is a key goal of nuclear astrophysics. Since these nuclei are unstable and neutron targets do not exist, performing these measurements require a facility that can produce the nuclei of interest at a sufficient rate to allow formation of a meaningful target (at least 1015 atoms). The Rare Isotope Accelerator (RIA) promises such rates, often enabling collection of greater than 1016 atoms after only of few days of production running. By properly designing both the ISOL and fragmentation lines, these collections will often be possible to obtained parasitically to other radioactive ion beam production. But given a target, performing the neutron capture cross-section measurement also presents its own challenges. In many cases, activation measurements are feasible, providing one obtains a target of sufficient purity. But for many branch point nuclei, the capture product is stable or long enough lived that no radiation signature is available for detection. Measurements for these nuclei will require a BaF2 array like DANCE at Los Alamos National Laboratory, which uses gamma calorimetry to detect neutron capture events. Plans and issues associated with isotope harvesting will be discussed, as well as challenges associated with performing theses measurements. Current plans for doing DANCE type measurements at RIA will also be discussed. This work was performed under the auspices of the U.S. Department of Energy by the University of California, Lawrence Livermore National Laboratory under contract No. W-7405-Eng-48.

  10. Quantization of Differences Between Atomic and Nuclear Rest Masses and Self-organization of Atoms and Nuclei

    NASA Astrophysics Data System (ADS)

    Gareev, F. A.; Zhidkova, I. E.

    2007-03-01

    We come to the conclusion that all atomic models based on either the Newton equation and the Kepler laws, or the Maxwell equations, or the Schrodinger and Dirac equations are in reasonable agreement with experimental data. We can only suspect that these equations are grounded on the same fundamental principle(s) which is (are) not known or these equations can be transformed into each other. We proposed a new mechanism of LENR: cooperative processes in the whole system nuclei + atoms + condensed matter - nuclear reactions in plasma - can occur at smaller threshold energies than the corresponding ones on free constituents. We were able to quantize phenomenologically the first time the differences between atomic and nuclear rest masses by the formula: δδM =n1/n2 X 0.0076294 (in MeV/ c^2), ni=1,2,3,.... Note that this quantization rule is justified for atoms and nuclei with different A, N and Z and the nuclei and atoms represent a coherent synchronized systems - a complex of coupled oscillators (resonators). The cooperative resonance synchronization mechanisms can explain how electron volt (atomic-) scale processes can induce and control nuclear MeV (nuclear-) scale processes and reactions., F.A. Gareev, I.E. Zhidkova, E-print arXiv Nucl-th/ 0610002 2006.

  11. Pion-less effective field theory for real and lattice nuclei

    NASA Astrophysics Data System (ADS)

    Bansal, Aaina; Binder, Sven; Ekström, Andreas; Hagen, Gaute; Papenbrock, Thomas

    2017-09-01

    We compute the medium-heavy nuclei 16O and 40Ca using pion-less effective field theory (EFT) at leading order (LO) and next-to-leading order (NLO). The low-energy coefficients of the EFT Hamiltonian are adjusted to A = 2 , 3 nuclei data from experiments, or alternatively to data from lattice QCD at unphysical pion mass mπ = 806 MeV. The EFT is implemented through discrete variable representation of finite harmonic oscillator basis. This approach ensures rapid convergence with respect to the size of the model space and allows us to compute heavier atomic and lattice nuclei. The atomic nuclei 16O and 40Ca are bound with respect to decay into alpha particles at NLO, but not at LO.

  12. Computational code in atomic and nuclear quantum optics: Advanced computing multiphoton resonance parameters for atoms in a strong laser field

    NASA Astrophysics Data System (ADS)

    Glushkov, A. V.; Gurskaya, M. Yu; Ignatenko, A. V.; Smirnov, A. V.; Serga, I. N.; Svinarenko, A. A.; Ternovsky, E. V.

    2017-10-01

    The consistent relativistic energy approach to the finite Fermi-systems (atoms and nuclei) in a strong realistic laser field is presented and applied to computing the multiphoton resonances parameters in some atoms and nuclei. The approach is based on the Gell-Mann and Low S-matrix formalism, multiphoton resonance lines moments technique and advanced Ivanov-Ivanova algorithm of calculating the Green’s function of the Dirac equation. The data for multiphoton resonance width and shift for the Cs atom and the 57Fe nucleus in dependence upon the laser intensity are listed.

  13. Vacuum low-temperature superconductivity is the essence of superconductivity - Atomic New Theory

    NASA Astrophysics Data System (ADS)

    Yongquan, Han

    2010-10-01

    The universe when the temperature closest to the Big Bang the temperature should be nuclear. Because, after the big bang, instant formation of atoms, nuclei and electrons between the absolute vacuum, the nucleus can not emit energy. (Radioactive elements, except in fact, radiation Yuan Su limited power emitted) which causes atomic nuclei and external temperature difference are so enormous that a large temperature difference reasons, all external particles became closer to the nucleus, affect the motion of electrons. When the conductor conductivity and thus affect the conductivity, the formation of resistance. Assumption that no particles affect the motion of electrons (except outside the nucleus) to form a potential difference will not change after the vector form, is now talking about the phenomenon of superconductivity, and then to introduce general, the gap between atoms in molecules or between small, valence electron number of high temperature superconducting conductors. This theory of atomic nuclei, but also explain the atomic and hydrogen bombs can remain after an explosion Why can release enormous energy reasons. Can also explain the ``super flow'' phenomenon. natural world. Tel 13241375685

  14. Experimental evidence of the decrease of kinetic energy of hadrons in passing through atomic nuclei

    NASA Technical Reports Server (NTRS)

    Strugalski, Z.

    1985-01-01

    Hadrons with kinetic energies higher than the pion production threshold lose their kinetic energies monotonically in traversing atomic nuclei, due to the strong interactions in nuclear matter. This phenomenon is a crude analogy to the energy loss of charged particles in their passage through materials. Experimental evidence is presented.

  15. Glass-wool study of laser-induced spin currents en route to hyperpolarized Cs salt

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Ishikawa, Kiyoshi

    2011-07-15

    The nuclear spin polarization of optically pumped Cs atoms flows to the surface of Cs hydride in a vapor cell. A fine glass wool lightly coated with the salt helps greatly increase the surface area in contact with the pumped atoms and enhance the spin polarization of the salt nuclei. Even though the glass wool randomly scatters the pump light, the atomic vapor can be polarized with unpolarized light in a magnetic field. The measured enhancement in the salt enables study of the polarizations of light and atomic nuclei very near the salt surface.

  16. Generalized vibrating potential model for collective excitations in spherical, deformed and superdeformed systems: (1) Atomic nuclei, (2) Metal clusters

    NASA Astrophysics Data System (ADS)

    Nesterenko, V. O.; Kleinig, W.

    1995-01-01

    The self-consistent vibrating potential model (VPM) is extended for description of Eλ collective excitations in atomic nuclei and metal clusters with practically any kind of static deformation. The model is convenient for a qualitative analysis and provides the RPA accuracy of numerical calculations. The VPM is applied to study Eλ giant resonances in spherical metal clusters and deformed and superdeformed nuclei. It is shown that the deformation splitting of superdeformed nuclei results in a very complicated ("jungle-like") structure of the resonances, which makes the experimental observation of E2 and E3 giant resonances in superdeformed nuclei quite problematic. Calculations of E1 giant resonances in spherical sodium clusters Na8, Na20 and Na40 are presented, as a test of the VPM in this field. The results are in qualitative agreement with the experimental data.

  17. Designer Nuclei--Making Atoms that Barely Exist

    ERIC Educational Resources Information Center

    Jones, Kate L.; Nazarewicz, Witold

    2010-01-01

    The physics of nuclei is not a democratic field. It has to be said, some nuclei are just more interesting than others. And some are more useful than others, either to explain the origins of the elements, or the nature of matter itself, or for uses in medicine and other applied fields. The trick is to work out which nuclei are going to be the most…

  18. Computer Model Of Fragmentation Of Atomic Nuclei

    NASA Technical Reports Server (NTRS)

    Wilson, John W.; Townsend, Lawrence W.; Tripathi, Ram K.; Norbury, John W.; KHAN FERDOUS; Badavi, Francis F.

    1995-01-01

    High Charge and Energy Semiempirical Nuclear Fragmentation Model (HZEFRG1) computer program developed to be computationally efficient, user-friendly, physics-based program for generating data bases on fragmentation of atomic nuclei. Data bases generated used in calculations pertaining to such radiation-transport applications as shielding against radiation in outer space, radiation dosimetry in outer space, cancer therapy in laboratories with beams of heavy ions, and simulation studies for designing detectors for experiments in nuclear physics. Provides cross sections for production of individual elements and isotopes in breakups of high-energy heavy ions by combined nuclear and Coulomb fields of interacting nuclei. Written in ANSI FORTRAN 77.

  19. Hidden momentum of electrons, nuclei, atoms, and molecules

    NASA Astrophysics Data System (ADS)

    Cameron, Robert P.; Cotter, J. P.

    2018-04-01

    We consider the positions and velocities of electrons and spinning nuclei and demonstrate that these particles harbour hidden momentum when located in an electromagnetic field. This hidden momentum is present in all atoms and molecules, however it is ultimately canceled by the momentum of the electromagnetic field. We point out that an electron vortex in an electric field might harbour a comparatively large hidden momentum and recognize the phenomenon of hidden hidden momentum.

  20. Foreword [Special Issue on Superheavy Elements

    DOE PAGES

    Düllmann, Christoph E.; Herzberg, Rolf -Dietmar; Nazarewicz, Witold; ...

    2015-12-07

    Reflecting the breadth of research opportunities in the field of superheavy element research, this special issue covers the range of topics in a comprehensive way, including synthesis of superheavy isotopes, nuclear structure, atomic shell structure, and chemical properties. The contributions detail the status of the field and lay out perspectives for the future. The prospects are bright: new isotopes are awaiting discovery, completing the landscape of superheavy nuclei and bridging the currently existing gap between nuclei synthesized in cold fusion reactions and those from 48Ca induced fusion reactions. The possibility that the limits of nuclear structure studies can be pushedmore » even further in mass and charge has greatly motivated a number of new facilities. Advances in experimental techniques will allow studies on isotopes produced significantly below the 1 pb level. Chemical studies progressing to elements never studied to date are already being prepared. Ultra-fast chemistry setups are under development and it will be fascinating to see them at work, elucidating the influence of relativistic effects on superheavy elements. The richness of chemical systems available for transactinides will expand further, giving access to new chemical systems, giving more information on the architecture of the periodic table.« less

  1. Nuclei and the Unitary Limit

    NASA Astrophysics Data System (ADS)

    Hammer, H.-W.

    2018-07-01

    Few-body systems with large scattering length display universal properties which are independent of the details of short-distance dynamics. These features include universal correlations between few-body observables and a geometric spectrum of three- and higher-body bound states. They can be observed in a wide range of systems from ultracold atoms to hadrons and nuclei. In this contribution, we review universality in nuclei dominated by few-body physics. In particular, we discuss halo nuclei and the description of light nuclei in a strict expansion around the unitary limit of infinite scattering length.

  2. Fundamental Studies of Crystal Growth of Microporous Materials

    NASA Technical Reports Server (NTRS)

    Singh, Ramsharan; Doolittle, John, Jr.; Payra, Pramatha; Dutta, Prabir K.; George, Michael A.; Ramachandran, Narayanan; Schoeman, Brian J.

    2003-01-01

    Microporous materials are framework structures with well-defined porosity, often of molecular dimensions. Zeolites contain aluminum and silicon atoms in their framework and are the most extensively studied amongst all microporous materials. Framework structures with P, Ga, Fe, Co, Zn, B, Ti and a host of other elements have also been made. Typical synthesis of microporous materials involve mixing the framework elements (or compounds, thereof) in a basic solution, followed by aging in some cases and then heating at elevated temperatures. This process is termed hydrothermal synthesis, and involves complex chemical and physical changes. Because of a limited understanding of this process, most synthesis advancements happen by a trial and error approach. There is considerable interest in understanding the synthesis process at a molecular level with the expectation that eventually new framework structures will be built by design. The basic issues in the microporous materials crystallization process include: (a) Nature of the molecular units responsible for the crystal nuclei formation; (b) Nature of the nuclei and nucleation process; (c) Growth process of the nuclei into crystal; (d) Morphological control and size of the resulting crystal; (e) Surface structure of the resulting crystals; and (f) Transformation of frameworks into other frameworks or condensed structures.

  3. Nuclear spectroscopy of r-process nuclei around N = 126 using KISS

    NASA Astrophysics Data System (ADS)

    Hirayama, Y.; Watanabe, Y. X.; Miyatake, H.; Schury, P.; Wada, M.; Oyaizu, M.; Kakiguchi, Y.; Mukai, M.; Kimura, S.; Ahmed, M.; Jeong, S. C.; Moon, J. Y.; Park, J. H.

    2017-09-01

    The beta-decay properties and atomic mass of nuclei with neutron magic number of N = 126 are considered critical for understanding the production of heavy elements such as gold and platinum at astrophysical sites. We will produce and measure the half-lives and masses of the nuclei with Z = 74-77 around N = 126 by using the multinucleon transfer (MNT) reaction of ^{136} Xe/ ^{238} U beams and ^{198} Pt target system. For this purpose, we have constructed the KEK Isotope Separation System (KISS) at RIKEN RIBF facility. KISS consists of an argon gas cell based laser ion source (atomic number selection) and an isotope separation on-line (ISOL) (mass number selection), to produce pure low-energy beams of neutron-rich isotopes around N = 126 . We performed the on-line tests to study the basic properties of the KISS and, successfully extracted laser-ionized nuclei around N = 126.

  4. Coupled-cluster computations of atomic nuclei

    NASA Astrophysics Data System (ADS)

    Hagen, G.; Papenbrock, T.; Hjorth-Jensen, M.; Dean, D. J.

    2014-09-01

    In the past decade, coupled-cluster theory has seen a renaissance in nuclear physics, with computations of neutron-rich and medium-mass nuclei. The method is efficient for nuclei with product-state references, and it describes many aspects of weakly bound and unbound nuclei. This report reviews the technical and conceptual developments of this method in nuclear physics, and the results of coupled-cluster calculations for nucleonic matter, and for exotic isotopes of helium, oxygen, calcium, and some of their neighbors.

  5. Effective field theory of emergent symmetry breaking in deformed atomic nuclei

    DOE PAGES

    Papenbrock, Thomas F.; Weidenmüller, H. A.

    2015-09-03

    Spontaneous symmetry breaking in non-relativistic quantum systems has previously been addressed in the framework of effective field theory. Low-lying excitations are constructed from Nambu–Goldstone modes using symmetry arguments only. In this study, we extend that approach to finite systems. The approach is very general. To be specific, however, we consider atomic nuclei with intrinsically deformed ground states. The emergent symmetry breaking in such systems requires the introduction of additional degrees of freedom on top of the Nambu–Goldstone modes. Symmetry arguments suffice to construct the low-lying states of the system. Lastly, in deformed nuclei these are vibrational modes each of whichmore » serves as band head of a rotational band.« less

  6. Systematics of ground state multiplets of atomic nuclei in the delta-interaction approach

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Imasheva, L. T.; Ishkhanov, B. S.; Stepanov, M. E., E-mail: stepanov@depni.sinp.msu.ru

    2015-12-15

    Pairing forces between nucleons in an atomic nucleus strongly influence its structure. One of the manifestations of pair interaction is the ground state multiplet (GSM) formation in the spectrum of low-lying excited states of even–even nuclei. The value of GSM splitting is determined by the value of pair interaction of nucleons; for each isotope, it can be estimated on the basis of experimental nuclear masses. The quality of this estimate is characterized by the degree of reproduction of GSM levels in the nucleus. The GSM systematics in even–even nuclei with a pair of identical nucleons in addition to the filledmore » nuclear core is considered on the basis of delta interaction.« less

  7. Deformation effect on spectral statistics of nuclei

    NASA Astrophysics Data System (ADS)

    Sabri, H.; Jalili Majarshin, A.

    2018-02-01

    In this study, we tried to get significant relations between the spectral statistics of atomic nuclei and their different degrees of deformations. To this aim, the empirical energy levels of 109 even-even nuclei in the 22 ≤ A ≤ 196 mass region are classified as their experimental and calculated quadrupole, octupole, hexadecapole and hexacontatetrapole deformations values and analyzed by random matrix theory. Our results show an obvious relation between the regularity of nuclei and strong quadrupole, hexadecapole and hexacontatetrapole deformations and but for nuclei that their octupole deformations are nonzero, we have observed a GOE-like statistics.

  8. Neutron and weak-charge distributions of the 48Ca nucleus

    DOE PAGES

    Hagen, Gaute; Forssen, Christian; Nazarewicz, Witold; ...

    2015-11-02

    What is the size of the atomic nucleus? This deceivably simple question is difficult to answer. Although the electric charge distributions in atomic nuclei were measured accurately already half a century ago, our knowledge of the distribution of neutrons is still deficient. In addition to constraining the size of atomic nuclei, the neutron distribution also impacts the number of nuclei that can exist and the size of neutron stars. We present an ab initio calculation of the neutron distribution of the neutron-rich nucleus 48Ca. We show that the neutron skin (difference between the radii of the neutron and proton distributions)more » is significantly smaller than previously thought. We also make predictions for the electric dipole polarizability and the weak form factor; both quantities that are at present targeted by precision measurements. Here, based on ab initio results for 48Ca, we provide a constraint on the size of a neutron star.« less

  9. Derivatives in discrete mathematics: a novel graph-theoretical invariant for generating new 2/3D molecular descriptors. I. Theory and QSPR application

    NASA Astrophysics Data System (ADS)

    Marrero-Ponce, Yovani; Santiago, Oscar Martínez; López, Yoan Martínez; Barigye, Stephen J.; Torrens, Francisco

    2012-11-01

    In this report, we present a new mathematical approach for describing chemical structures of organic molecules at atomic-molecular level, proposing for the first time the use of the concept of the derivative ( partial ) of a molecular graph (MG) with respect to a given event ( E), to obtain a new family of molecular descriptors (MDs). With this purpose, a new matrix representation of the MG, which generalizes graph's theory's traditional incidence matrix, is introduced. This matrix, denominated the generalized incidence matrix, Q, arises from the Boolean representation of molecular sub- graphs that participate in the formation of the graph molecular skeleton MG and could be complete (representing all possible connected sub-graphs) or constitute sub-graphs of determined orders or types as well as a combination of these. The Q matrix is a non-quadratic and unsymmetrical in nature, its columns ( n) and rows ( m) are conditions (letters) and collection of conditions (words) with which the event occurs. This non-quadratic and unsymmetrical matrix is transformed, by algebraic manipulation, to a quadratic and symmetric matrix known as relations frequency matrix, F, which characterizes the participation intensity of the conditions (letters) in the events (words). With F, we calculate the derivative over a pair of atomic nuclei. The local index for the atomic nuclei i, Δ i , can therefore be obtained as a linear combination of all the pair derivatives of the atomic nuclei i with all the rest of the j's atomic nuclei. Here, we also define new strategies that generalize the present form of obtaining global or local (group or atom-type) invariants from atomic contributions (local vertex invariants, LOVIs). In respect to this, metric (norms), means and statistical invariants are introduced. These invariants are applied to a vector whose components are the values Δ i for the atomic nuclei of the molecule or its fragments. Moreover, with the purpose of differentiating among different atoms, an atomic weighting scheme (atom-type labels) is used in the formation of the matrix Q or in LOVIs state. The obtained indices were utilized to describe the partition coefficient (Log P) and the reactivity index (Log K) of the 34 derivatives of 2-furylethylenes. In all the cases, our MDs showed better statistical results than those previously obtained using some of the most used families of MDs in chemometric practice. Therefore, it has been demonstrated to that the proposed MDs are useful in molecular design and permit obtaining easier and robust mathematical models than the majority of those reported in the literature. All this range of mentioned possibilities open "the doors" to the creation of a new family of MDs, using the graph derivative, and avail a new tool for QSAR/QSPR and molecular diversity/similarity studies.

  10. Derivatives in discrete mathematics: a novel graph-theoretical invariant for generating new 2/3D molecular descriptors. I. Theory and QSPR application.

    PubMed

    Marrero-Ponce, Yovani; Santiago, Oscar Martínez; López, Yoan Martínez; Barigye, Stephen J; Torrens, Francisco

    2012-11-01

    In this report, we present a new mathematical approach for describing chemical structures of organic molecules at atomic-molecular level, proposing for the first time the use of the concept of the derivative ([Formula: see text]) of a molecular graph (MG) with respect to a given event (E), to obtain a new family of molecular descriptors (MDs). With this purpose, a new matrix representation of the MG, which generalizes graph's theory's traditional incidence matrix, is introduced. This matrix, denominated the generalized incidence matrix, Q, arises from the Boolean representation of molecular sub-graphs that participate in the formation of the graph molecular skeleton MG and could be complete (representing all possible connected sub-graphs) or constitute sub-graphs of determined orders or types as well as a combination of these. The Q matrix is a non-quadratic and unsymmetrical in nature, its columns (n) and rows (m) are conditions (letters) and collection of conditions (words) with which the event occurs. This non-quadratic and unsymmetrical matrix is transformed, by algebraic manipulation, to a quadratic and symmetric matrix known as relations frequency matrix, F, which characterizes the participation intensity of the conditions (letters) in the events (words). With F, we calculate the derivative over a pair of atomic nuclei. The local index for the atomic nuclei i, Δ(i), can therefore be obtained as a linear combination of all the pair derivatives of the atomic nuclei i with all the rest of the j's atomic nuclei. Here, we also define new strategies that generalize the present form of obtaining global or local (group or atom-type) invariants from atomic contributions (local vertex invariants, LOVIs). In respect to this, metric (norms), means and statistical invariants are introduced. These invariants are applied to a vector whose components are the values Δ(i) for the atomic nuclei of the molecule or its fragments. Moreover, with the purpose of differentiating among different atoms, an atomic weighting scheme (atom-type labels) is used in the formation of the matrix Q or in LOVIs state. The obtained indices were utilized to describe the partition coefficient (Log P) and the reactivity index (Log K) of the 34 derivatives of 2-furylethylenes. In all the cases, our MDs showed better statistical results than those previously obtained using some of the most used families of MDs in chemometric practice. Therefore, it has been demonstrated to that the proposed MDs are useful in molecular design and permit obtaining easier and robust mathematical models than the majority of those reported in the literature. All this range of mentioned possibilities open "the doors" to the creation of a new family of MDs, using the graph derivative, and avail a new tool for QSAR/QSPR and molecular diversity/similarity studies.

  11. Heaviest Nuclei: New Element with Atomic Number 117

    ScienceCinema

    Oganessian, Yuri

    2018-01-24

    One of the fundamental outcomes of the nuclear shell model is the prediction of the 'stability islands' in the domain of the hypothetical super heavy elements. The talk is devoted to the experimental verification of these predictions - the synthesis and study of both the decay and chemical properties of the super heavy elements. The discovery of a new chemical element with atomic number Z=117 is reported. The isotopes 293117 and 294117 were produced in fusion reactions between 48Ca and 249Bk. Decay chains involving 11 new nuclei were identified by means of the Dubna gas-filled recoil separator. The measured decay properties show a strong rise of stability for heavier isotopes with Z =111, validating the concept of the long sought island of enhanced stability for heaviest nuclei.

  12. Colloquium: Laser probing of neutron-rich nuclei in light atoms

    NASA Astrophysics Data System (ADS)

    Lu, Z.-T.; Mueller, P.; Drake, G. W. F.; Nörtershäuser, W.; Pieper, Steven C.; Yan, Z.-C.

    2013-10-01

    The neutron-rich He6 and He8 isotopes exhibit an exotic nuclear structure that consists of a tightly bound He4-like core with additional neutrons orbiting at a relatively large distance, forming a halo. Recent experimental efforts have succeeded in laser trapping and cooling these short-lived, rare helium atoms and have measured the atomic isotope shifts along the He4-He6-He8 chain by performing laser spectroscopy on individual trapped atoms. Meanwhile, the few-electron atomic structure theory, including relativistic and QED corrections, has reached a comparable degree of accuracy in the calculation of the isotope shifts. In parallel efforts, also by measuring atomic isotope shifts, the nuclear charge radii of lithium and beryllium isotopes have been studied. The techniques employed were resonance ionization spectroscopy on neutral, thermal lithium atoms and collinear laser spectroscopy on beryllium ions. Combining advances in both atomic theory and laser spectroscopy, the charge radii of these light halo nuclei have now been determined for the first time independent of nuclear structure models. The results are compared with the values predicted by a number of nuclear structure calculations and are used to guide our understanding of the nuclear forces in the extremely neutron-rich environment.

  13. Predictions of nuclear charge radii

    NASA Astrophysics Data System (ADS)

    Bao, M.; Lu, Y.; Zhao, Y. M.; Arima, A.

    2016-12-01

    The nuclear charge radius is a fundamental property of an atomic nucleus. In this article we study the predictive power of empirical relations for experimental nuclear charge radii of neighboring nuclei and predict the unknown charge radii of 1085 nuclei based on the experimental CR2013 database within an uncertainty of 0.03 fm.

  14. The Atomic Mass Evaluation (AME2012): Status and Perspectives

    NASA Astrophysics Data System (ADS)

    Kondev, F. G.; Audi, G.; Wang, M.; Xu, X.; Wapstra, A. H.; MacCormick, M.; Pfeiffer, B.

    2013-10-01

    The atomic mass is a fundamental property of the nucleus that has wide applications in natural sciences and technology. The new evaluated mass table, AME2012, has been recently published as a collaborative effort between scientists from China, Europe and USA, under the leadership of G. Audi. It represents a significant update of the previous AME2003 evaluation by considering a large number of precise experimental results obtained at existing Penning Trap and Storage Ring facilities, thus expending the region of experimentally known masses towards exotic neutron- and proton-rich nuclei. Since the presence of isomers plays an important role in determining the masses of many nuclei, a complementary database, NUBASE2012, that contains the isomer-level properties for all nuclei was also developed. This presentation will briefly review recent achievements of the collaboration, present on-going activities, and reflect on ideas for future developments and challenges in the field of evaluation of atomic masses. The work at ANL was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357.

  15. Calculations of long-range three-body interactions for He(n0λS )-He(n0λS )-He(n0'λL )

    NASA Astrophysics Data System (ADS)

    Yan, Pei-Gen; Tang, Li-Yan; Yan, Zong-Chao; Babb, James F.

    2018-04-01

    We theoretically investigate long-range interactions between an excited L -state He atom and two identical S -state He atoms for the cases of the three atoms all in spin-singlet states or all in spin-triplet states, denoted by He(n0λS )-He(n0λS )-He(n0'λL ), with n0 and n0' principal quantum numbers, λ =1 or 3 the spin multiplicity, and L the orbital angular momentum of a He atom. Using degenerate perturbation theory for the energies up to second-order, we evaluate the coefficients C3 of the first-order dipolar interactions and the coefficients C6 and C8 of the second-order additive and nonadditive interactions. Both the dipolar and dispersion interaction coefficients, for these three-body degenerate systems, show dependences on the geometrical configurations of the three atoms. The nonadditive interactions start to appear in second-order. To demonstrate the results and for applications, the obtained coefficients Cn are evaluated with highly accurate variationally generated nonrelativistic wave functions in Hylleraas coordinates for He(1 1S ) -He(1 1S ) -He(2 1S ) , He(1 1S ) -He(1 1S ) -He(2 1P ) , He(2 1S ) -He(2 1S ) -He(2 1P ) , and He(2 3S ) -He(2 3S ) -He(2 3P ) . The calculations are given for three like nuclei for the cases of hypothetical infinite mass He nuclei, and of real finite mass 4He or 3He nuclei. The special cases of the three atoms in equilateral triangle configurations are explored in detail, and for the cases in which one of the atoms is in a P state, we also present results for the atoms in an isosceles right triangle configuration or in an equally spaced collinear configuration. The results can be applied to construct potential energy surfaces for three helium atom systems.

  16. Effective field theory for deformed atomic nuclei

    DOE PAGES

    Papenbrock, Thomas F.; Weidenmüller, H. A.

    2016-04-13

    In this paper, we present an effective field theory (EFT) for a model-independent description of deformed atomic nuclei. In leading order this approach recovers the well-known results from the collective model by Bohr and Mottelson. When higher-order corrections are computed, the EFT accounts for finer details such as the variation of the moment of inertia with the band head and the small magnitudes of interband E2 transitions. Finally, for rotational bands with a finite spin of the band head, the EFT is equivalent to the theory of a charged particle on the sphere subject to a magnetic monopole field.

  17. The abundances of solar accelerated nuclei from carbon to iron.

    NASA Technical Reports Server (NTRS)

    Mogro-Campero, A.; Simpson, J. A.

    1972-01-01

    Revised observation periods and new data are found to confirm previous evidence that the overabundance of solar-flare nuclei with respect to solar photospheric and coronal abundances increases with increasing atomic number. It is also verified that enhancements can vary from flare to flare and that this variability is large enough to explain the differences observed by various investigators regarding the magnitude of solar-flare high-Z particle enhancements. Additional evidence for a two-stage solar acceleration mechanism is obtained. It is shown that the galactic cosmic-ray source composition displays a similar overabundance as a function of atomic number.

  18. Fundamental Studies of Crystal Growth of Microporous Materials

    NASA Technical Reports Server (NTRS)

    Dutta, P.; George, M.; Ramachandran, N.; Schoeman, B.; Curreri, Peter A. (Technical Monitor)

    2002-01-01

    Microporous materials are framework structures with well-defined porosity, often of molecular dimensions. Zeolites contain aluminum and silicon atoms in their framework and are the most extensively studied amongst all microporous materials. Framework structures with P, Ga, Fe, Co, Zn, B, Ti and a host of other elements have also been made. Typical synthesis of microporous materials involve mixing the framework elements (or compounds, thereof) in a basic solution, followed by aging in some cases and then heating at elevated temperatures. This process is termed hydrothermal synthesis, and involves complex chemical and physical changes. Because of a limited understanding of this process, most synthesis advancements happen by a trial and error approach. There is considerable interest in understanding the synthesis process at a molecular level with the expectation that eventually new framework structures will be built by design. The basic issues in the microporous materials crystallization process include: (1) Nature of the molecular units responsible for the crystal nuclei formation; (2) Nature of the nuclei and nucleation process; (3) Growth process of the nuclei into crystal; (4) Morphological control and size of the resulting crystal; (5) Surface structure of the resulting crystals; (6) Transformation of frameworks into other frameworks or condensed structures. The NASA-funded research described in this report focuses to varying degrees on all of the above issues and has been described in several publications. Following is the presentation of the highlights of our current research program. The report is divided into five sections: (1) Fundamental aspects of the crystal growth process; (2) Morphological and Surface properties of crystals; (3) Crystal dissolution and transformations; (4) Modeling of Crystal Growth; (5) Relevant Microgravity Experiments.

  19. Process-Structure-Property Relationships of Micron Thick Gadolinium Oxide Films Deposited by Reactive Electron Beam-Physical Vapor Deposition (EB-PVD)

    DTIC Science & Technology

    2014-12-01

    surface roughness on film properties must be considered. Stability at the interface between the film and the substrate becomes critical with...etc.). Addition of atoms to the growing surface creates additional surface energy. Therefore, nuclei of a critical size 23 must be formed in order... critical nuclei size and a lower nucleation rate. Higher deposition rates result in a decreased critical nuclei size which leads to an increase in

  20. In situ mechanical characterization of the cell nucleus by atomic force microscopy.

    PubMed

    Liu, Haijiao; Wen, Jun; Xiao, Yun; Liu, Jun; Hopyan, Sevan; Radisic, Milica; Simmons, Craig A; Sun, Yu

    2014-04-22

    The study of nuclear mechanical properties can provide insights into nuclear dynamics and its role in cellular mechanotransduction. While several methods have been developed to characterize nuclear mechanical properties, direct intracellular probing of the nucleus in situ is challenging. Here, a modified AFM (atomic force microscopy) needle penetration technique is demonstrated to mechanically characterize cell nuclei in situ. Cytoplasmic and nuclear stiffness were determined based on two different segments on the AFM indentation curves and were correlated with simultaneous confocal Z-stack microscopy reconstructions. On the basis of direct intracellular measurement, we show that the isolated nuclei from fibroblast-like cells exhibited significantly lower Young's moduli than intact nuclei in situ. We also show that there is in situ nucleus softening in the highly metastatic bladder cancer cell line T24 when compared to its less metastatic counterpart RT4. This technique has potential to become a reliable quantitative measurement tool for intracellular mechanics studies.

  1. Nuclear physics (of the cell, not the atom).

    PubMed

    Pederson, Thoru; Marko, John F

    2014-11-05

    The nucleus is physically distinct from the cytoplasm in ways that suggest new ideas and approaches for interrogating the operation of this organelle. Chemical bond formation and breakage underlie the lives of cells, but as this special issue of Molecular Biology of the Cell attests, the nonchemical aspects of cell nuclei present a new frontier to biologists and biophysicists. © 2014 Pederson and Marko. This article is distributed by The American Society for Cell Biology under license from the author(s). Two months after publication it is available to the public under an Attribution–Noncommercial–Share Alike 3.0 Unported Creative Commons License (http://creativecommons.org/licenses/by-nc-sa/3.0).

  2. Extending DFT-based genetic algorithms by atom-to-place re-assignment via perturbation theory: A systematic and unbiased approach to structures of mixed-metallic clusters

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Weigend, Florian, E-mail: florian.weigend@kit.edu

    2014-10-07

    Energy surfaces of metal clusters usually show a large variety of local minima. For homo-metallic species the energetically lowest can be found reliably with genetic algorithms, in combination with density functional theory without system-specific parameters. For mixed-metallic clusters this is much more difficult, as for a given arrangement of nuclei one has to find additionally the best of many possibilities of assigning different metal types to the individual positions. In the framework of electronic structure methods this second issue is treatable at comparably low cost at least for elements with similar atomic number by means of first-order perturbation theory, asmore » shown previously [F. Weigend, C. Schrodt, and R. Ahlrichs, J. Chem. Phys. 121, 10380 (2004)]. In the present contribution the extension of a genetic algorithm with the re-assignment of atom types to atom sites is proposed and tested for the search of the global minima of PtHf{sub 12} and [LaPb{sub 7}Bi{sub 7}]{sup 4−}. For both cases the (putative) global minimum is reliably found with the extended technique, which is not the case for the “pure” genetic algorithm.« less

  3. Lamb shift and fine structure at n =2 in a hydrogenlike muonic atom with the nuclear spin I =0

    NASA Astrophysics Data System (ADS)

    Korzinin, Evgeny Yu.; Shelyuto, Valery A.; Ivanov, Vladimir G.; Karshenboim, Savely G.

    2018-01-01

    The paper is devoted to the Lamb shift and fine structure in a hydrogenlike muonic atom with a spinless nucleus up to the order α5m with all the recoil corrections included. Enhanced contributions of a higher order are also considered. We present the results on the pure QED contribution and on the finite-nuclear-size contribution, proportional to RN2, with the higher-order corrections included. We also consider the consistency of the pure QED theory and the evaluation of the nuclear-structure effects. Most of the QED theory is the same as the theory for the case of the nuclear spin 1/2. Additional nuclear-spin-dependent terms are considered in detail. The issue of the difference for the theories with a spinor nucleus and a scalar one is discussed for the recoil contributions in the order (Zα ) 4m ,α (Zα ) 4m , and (Zα ) 5m . The numerical results are presented for the muonic atoms with two lightest scalar nuclei, helium-4 and beryllium-10. We compare the theory of those muonic atoms with theory for the muonic hydrogen. Some higher-order finite-nuclear-size corrections for the Lamb shift in muonic hydrogen are revisited.

  4. Delayed fission of atomic nuclei (To the 50th anniversary of the discovery)

    NASA Astrophysics Data System (ADS)

    Skobelev, N. K.

    2017-09-01

    The history of the discovery of delayed nuclear fission is presented, and the retrospective of investigations into this phenomenon that were performed at various research centers worldwide is outlined. The results obtained by measuring basic delayed-fission features, including the fission probability, the total kinetic energy of fission fragments, and their mass distributions, are analyzed. Recommendations concerning further studies in various regions of nuclear map with the aim of searches for and investigation of atomic nuclei undergoing delayed fission are given. Lines of further research into features of delayed fission with the aim of solving current problems of fission physics are discussed.

  5. Fusion barrier characteristics of actinides

    NASA Astrophysics Data System (ADS)

    Manjunatha, H. C.; Sridhar, K. N.

    2018-03-01

    We have studied fusion barrier characteristics of actinide compound nuclei with atomic number range 89 ≤ Z ≤ 103 for all projectile target combinations. After the calculation of fusion barrier heights and positions, we have searched for their parameterization. We have achieved the empirical formula for fusion barrier heights (VB), positions (RB), curvature of the inverted parabola (ħω) of actinide compound nuclei with atomic number range 89 ≤ Z ≤ 103 for all projectile target combinations (6

  6. Isomorphic Properties of Atoms, Molecules, Water, DNA, Crystals, Earth, SolarSystem and Galaxies

    NASA Astrophysics Data System (ADS)

    Gareev, F. A.; Gareeva, G. F.; Zhidkova, I. E.

    2009-03-01

    We discuss the cooperative resonance synchronization enhancement mechanisms of Low Energy Nuclear Reactions (LENR). Some of the low energy external fields can be used as triggers for starting and enhancing exothermic LENR. Any external field shortening distances between protons in nuclei and electrons in atoms should enhance beta-decay (capture) or double-beta decay (capture). We have proposed a new mechanism of LENR: cooperative resonance synchronization processes in the whole system nuclei+atoms+condensed matter+gaseuos+plasma medium, which we suggest can occur at a smaller threshold than the corresponding ones on free constituents. The cooperative processes can be induced and enhanced by low energy external fields. The excess heat is the emission of internal energy, and transmutations at LENR are the result of redistribution inner energy of the whole system.

  7. Study of crystallization mechanisms of Fe nanoparticle

    NASA Astrophysics Data System (ADS)

    Kien, P. H.; Trang, G. T. T.; Hung, P. K.

    2017-06-01

    In this paper, the nanoparticle (NP) Fe was investigated by means of molecular dynamics simulation. The crystallization mechanism was studied through the time evolution of crystal cluster and potential energies of different atom types. The simulation shows that the NP was crystallized into bcc crystal structure when it was annealed at 900 K for long times. At early stage of the annealing, small nuclei form in different places of NP and dissolve for short times. After long times some nuclei form and gather nearby which create the stable clusters in the core of NP. After that the crystal clusters grow in the direction to cover the core and then to spread into the surface of NP. Analyzing the energies of different type atoms, we found that the crystal growth is originated from specific atomic arrangement in the boundary region of crystal clusters.

  8. Synthesis reactions and radioactive properties of transactinoid elements

    NASA Astrophysics Data System (ADS)

    Oganessian, Yu. Ts.

    1994-10-01

    It is well known that the heaviest elements of the periodic table have been synthesized in the cold fusion of magic nuclei of Pb with Z less than 26 ions. Because of dynamic limitations for fusion under strong Coulomb interaction of nuclei, the cross-sections of cold fusion reactions diminish exponentially with growing compound nucleus atomic number. For element Z = 110 produced in the reaction Pb-208(Ni-62,n)(sub 271)110, the expected cross-section is 10(exp -36) sq cm. In still more asymmetric reactions, when isotopes of actinoid elements irradiated with relatively light ions (Z less than or equal 12) are used as the target material, the compound nuclei possess an excitation energy of approx. 50 MeV. At this energy the nuclear shell effects are strongly suppressed and, as a result, in the case of hot compound nuclei of transactinoid elements the fission barrier is practically absent. The transition of these nuclei into the ground state depends strongly on the dynamic properties of the system with respect to the fission degree of freedom. Experimental studies were going on in two directions: (1) determination of the fission time by measuring the prefission neutrons (of Cf-Fm nuclei) in a wide interval of excitation energies; (2) direct synthesis of known nuclides with Z = 102-105 in reactions with ions of Ne-22, Mg-26, Al-27 and P-31 when final nuclei are produced in the ground state after the evaporation of five or six neutrons from the excited compound nuclei (E(sub x) = 50-60 MeV). The dependence of the reaction cross-section (HI, 5-6n) on the atomic number of the compound nucleus in different target-ion combinations points to the possibility of synthesizing new elements in hot fusion reactions. The advantage of these reactions arises from the use of neutron-rich nuclei like Cm-248 and Cf-249 which allows us to synthesize nuclei close to the deformed shell N = 162, for which a considerable growth of stability against spontaneous fission is predicted. Experimental set-ups and methods of detecting rare events of formation and decay of transactinide nuclei are described.

  9. Influence of orbital symmetry on diffraction imaging with rescattering electron wave packets

    DOE PAGES

    Pullen, M. G.; Wolter, B.; Le, A. -T.; ...

    2016-06-22

    The ability to directly follow and time-resolve the rearrangement of the nuclei within molecules is a frontier of science that requires atomic spatial and few-femtosecond temporal resolutions. While laser-induced electron diffraction can meet these requirements, it was recently concluded that molecules with particular orbital symmetries (such as pg) cannot be imaged using purely backscattering electron wave packets without molecular alignment. Here, we demonstrate, in direct contradiction to these findings, that the orientation and shape of molecular orbitals presents no impediment for retrieving molecular structure with adequate sampling of the momentum transfer space. We overcome previous issues by showcasing retrieval ofmore » the structure of randomly oriented O 2 and C 2H 2 molecules, with π g and π u symmetries, respectively, and where their ionization probabilities do not maximize along their molecular axes. As a result, while this removes a serious bottleneck for laser-induced diffraction imaging, we find unexpectedly strong backscattering contributions from low-Z atoms.« less

  10. Gravitational waves from neutron stars and asteroseismology.

    PubMed

    Ho, Wynn C G

    2018-05-28

    Neutron stars are born in the supernova explosion of massive stars. Neutron stars rotate as stably as atomic clocks and possess densities exceeding that of atomic nuclei and magnetic fields millions to billions of times stronger than those created in laboratories on the Earth. The physical properties of neutron stars are determined by many areas of fundamental physics, and detection of gravitational waves can provide invaluable insights into our understanding of these areas. Here, we describe some of the physics and astrophysics of neutron stars and how traditional electromagnetic wave observations provide clues to the sorts of gravitational waves we expect from these stars. We pay particular attention to neutron star fluid oscillations, examining their impact on electromagnetic and gravitational wave observations when these stars are in a wide binary or isolated system, then during binary inspiral right before merger, and finally at times soon after merger.This article is part of a discussion meeting issue 'The promises of gravitational-wave astronomy'. © 2018 The Author(s).

  11. Gravitational waves from neutron stars and asteroseismology

    NASA Astrophysics Data System (ADS)

    Ho, Wynn C. G.

    2018-05-01

    Neutron stars are born in the supernova explosion of massive stars. Neutron stars rotate as stably as atomic clocks and possess densities exceeding that of atomic nuclei and magnetic fields millions to billions of times stronger than those created in laboratories on the Earth. The physical properties of neutron stars are determined by many areas of fundamental physics, and detection of gravitational waves can provide invaluable insights into our understanding of these areas. Here, we describe some of the physics and astrophysics of neutron stars and how traditional electromagnetic wave observations provide clues to the sorts of gravitational waves we expect from these stars. We pay particular attention to neutron star fluid oscillations, examining their impact on electromagnetic and gravitational wave observations when these stars are in a wide binary or isolated system, then during binary inspiral right before merger, and finally at times soon after merger. This article is part of a discussion meeting issue `The promises of gravitational-wave astronomy'.

  12. On the Mass of Atoms in Molecules: Beyond the Born-Oppenheimer Approximation

    NASA Astrophysics Data System (ADS)

    Scherrer, Arne; Agostini, Federica; Sebastiani, Daniel; Gross, E. K. U.; Vuilleumier, Rodolphe

    2017-07-01

    Describing the dynamics of nuclei in molecules requires a potential energy surface, which is traditionally provided by the Born-Oppenheimer or adiabatic approximation. However, we also need to assign masses to the nuclei. There, the Born-Oppenheimer picture does not account for the inertia of the electrons, and only bare nuclear masses are considered. Nowadays, experimental accuracy challenges the theoretical predictions of rotational and vibrational spectra and requires the participation of electrons in the internal motion of the molecule. More than 80 years after the original work of Born and Oppenheimer, this issue has still not been solved, in general. Here, we present a theoretical and numerical framework to address this problem in a general and rigorous way. Starting from the exact factorization of the electron-nuclear wave function, we include electronic effects beyond the Born-Oppenheimer regime in a perturbative way via position-dependent corrections to the bare nuclear masses. This maintains an adiabaticlike point of view: The nuclear degrees of freedom feel the presence of the electrons via a single potential energy surface, whereas the inertia of electrons is accounted for and the total mass of the system is recovered. This constitutes a general framework for describing the mass acquired by slow degrees of freedom due to the inertia of light, bounded particles; thus, it is applicable not only in electron-nuclear systems but in light-heavy nuclei or ions as well. We illustrate this idea with a model of proton transfer, where the light particle is the proton and the heavy particles are the oxygen atoms to which the proton is bounded. Inclusion of the light-particle inertia allows us to gain orders of magnitude in accuracy. The electron-nuclear perspective is adopted, instead, to calculate position-dependent mass corrections using density functional theory for a few polyatomic molecules at their equilibrium geometry. These data can serve as input for the computation of high-precision molecular spectra.

  13. Learning Nuclear Science with Marbles

    ERIC Educational Resources Information Center

    Constan, Zach

    2010-01-01

    Nuclei are "small": if an atom was the size of a football field, the nucleus would be an apple sitting on the 50-yd line. At the same time, nuclei are "dense": the Earth, compressed to nuclear density, could fit inside four Sears Towers. The subatomic level is strange and exotic. For that reason, it's not hard to get young minds excited about…

  14. The project of the mass separator of atomic nuclei produced in heavy ion induced reactions

    NASA Astrophysics Data System (ADS)

    Oganessian, Yu. Ts.; Shchepunov, V. A.; Dmitriev, S. N.; Itkis, M. G.; Gulbekyan, G. G.; Khabarov, M. V.; Bekhterev, V. V.; Bogomolov, S. L.; Efremov, A. A.; Pashenko, S. V.; Stepantsov, S. V.; Yeremin, A. V.; Yavor, M. I.; Kalimov, A. G.

    2003-05-01

    A new separator and mass analyzer, named MASHA (mass analyzer of super heavy atoms), has been designed at the Flerov Laboratory JINR Dubna to separate and measure masses of nuclei and molecules with precision better than 10 -3. The set up can work in the wide mass range from A≈20 to A≈500, its mass acceptance is as large as ±2.8%. In particular, it allows unambiguous mass identification of super heavy nuclei with a resolution better than 1 amu at the level of 300 amu. Synthesized in nuclear reactions nuclides are emitted from an ECR ion source at energy E=40 kV and charge state Q=+1. Then they pass the following steps of separation and analysis: the first section of rough separation, the second section of separation and mass analysis and the final section of separation with a 90° electrostatic deflector. In the focal plane of the device, a focal plane detector determines positions (masses) of studied nuclei. Ion optics of the analyzer, optimized up to the second order, is considered. Description of its elements and subsystems is given.

  15. Realistic Gamow shell model for resonance and continuum in atomic nuclei

    NASA Astrophysics Data System (ADS)

    Xu, F. R.; Sun, Z. H.; Wu, Q.; Hu, B. S.; Dai, S. J.

    2018-02-01

    The Gamow shell model can describe resonance and continuum for atomic nuclei. The model is established in the complex-moment (complex-k) plane of the Berggren coordinates in which bound, resonant and continuum states are treated on equal footing self-consistently. In the present work, the realistic nuclear force, CD Bonn, has been used. We have developed the full \\hat{Q}-box folded-diagram method to derive the realistic effective interaction in the model space which is nondegenerate and contains resonance and continuum channels. The CD-Bonn potential is renormalized using the V low-k method. With choosing 16O as the inert core, we have applied the Gamow shell model to oxygen isotopes.

  16. Nuclear choices

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Wolfson, R.

    This book contains part of the series New Liberal Arts, which is intended to make science and technology more accessible to students of the liberal arts. Volume in hand provides a comprehensive, multifaceted examination of nuclear energy, in nontechnical terms. Wolfson explains the basics of nuclear energy and radiation, nuclear power..., and nuclear weapons..., and he invites readers to make their own judgments on controversial nuclear issues. Illustrated with photos and diagrams. Each chapter contains suggestions for additional reading and a glossary. For policy, science, and general collections in all libraries. (ES) Topics contained include Atoms and nuclei. Effects andmore » uses of radiation. Energy and People. Reactor safety. Nuclear strategy. Defense in the nuclear age. Nuclear power, nuclear weapons, and nuclear futures.« less

  17. The P-factor and atomic mass systematics: Application to medium mass nuclei

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Brenner, D.S.; Haustein, P.E.; Casten, R.F.

    1988-01-01

    The P formalism was applied to atomic mass systematics for medium and heavy nuclei. The P-factor linearizes the structure-dependent part of the nuclear mass in those regions which are free from subshell effects indicating that the attractive quadrupole p-n force plays an important role in determining the binding of valence nucleons. Where marked non-linearities occur, the P-factor provides a means for recognizing subshell closures and/or other structural features not embodied in the simple assumptions of abrupt shell or subshell changes. These are thought to be regions where the monopole part of the p-n interaction is highly orbit dependent and altersmore » the underlying single-particle structure as a function of A, N or Z. Finally, in those regions where the systematics are smooth and subshells are absent, the P-factor provides a means for predicting masses of some nuclei far-from-stability by interpolation rather than by extrapolation. 5 figs.« less

  18. Muon, photon and nuclear CERs for ββ - ν response studies

    NASA Astrophysics Data System (ADS)

    Ejiri, H.

    2015-10-01

    Neutrino nuclear responses for neutrino-less double beta decays (0νββ DBD) are studied by muon, photon and nuclear charge exchange reactions (CER) and β-EC transitions. These experimental responses with low and medium momentum transfers are used to evaluate 0νββ nuclear matrix elements and the solar neutrino interactions with atoms and nuclei of DBD detectors. Gamma-ray measurements from residual RI nuclei produced by (µ, νµxn) reactions on 100Mo shows a giant resonance around 12-15 MeV for µ- capture strength. Single β Gamow-Teller (GT) and spin-dipole (SD) strengths are reduced with respect to pnQRPA calculations by gAe f f≈0.5 -0.6 gA , suggesting considerable reductions of the axial vector responses for DBD. Solar neutrino nuclear interactions with nuclei of the DBD isotopes and atoms of liquid scintillators used for DBD experiments are shown to be the serious backgrounds at the ROI (region of interest) of 0νββ.

  19. Enrichment of heavy nuclei in He-3-rich flares. [Imp-7 observed solar events

    NASA Technical Reports Server (NTRS)

    Hurford, G. J.; Mewaldt, R. A.; Stone, E. C.; Vogt, R. E.

    1975-01-01

    IMP-7 observations of five solar-flare particle events characterized by He-3 enrichment are reported which show that such events are also enriched in nuclei with charges (Z) of at least 6. The ratio of these nuclei to H-1 at approximately 3 MeV/nucleon was found to be enriched by about 10 to 100 times, while the ratio with respect to He-4 was enriched by about 3 to 30 times. It is suggested that the simultaneous enhancement of He-3 and the heavier nuclei as well as the absence of H-2 and H-3 during the observed events may be partly due to a preferential acceleration process which depends on the ratio of the square of the charge to the atomic weight of the nuclei.

  20. High baryon densities in heavy ion collisions at energies attainable at the BNL Relativistic Heavy-Ion Collider and the CERN Large Hadron Collider

    NASA Astrophysics Data System (ADS)

    Li, Ming; Kapusta, Joseph I.

    2017-01-01

    In very high-energy collisions nuclei are practically transparent to each other but produce very hot nearly baryon-free matter in the so-called central rapidity region. The energy in the central rapidity region comes from the kinetic energy of the colliding nuclei. We calculate the energy and rapidity loss of the nuclei using the color glass condensate model. This model also predicts the excitation energy of the nuclear fragments. Using a space-time picture of the collision we calculate the baryon and energy densities of the receding baryonic fireballs. For central collisions of gold nuclei at the highest energy attainable at the Relativistic Heavy-Ion Collider, for example, we find baryon densities more than ten times that of atomic nuclei over a large volume.

  1. Structural and compositional evolution of Al{sub 3}(Zr,Y) precipitates in Al-Zr-Y alloy

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Gao, Haiyan, E-mail: gaohaiyan@sjtu.edu.cn

    Structural and compositional evolution of Al{sub 3}(Zr,Y) precipitates in aged Al-Zr-Y alloy was investigated through atom probe tomography (APT) and transmission electron microscope (TEM) analysis and first principles calculations. The results show that short-bar-shaped D0{sub 19}-Al{sub 3}Y with some Zr atoms dissolved in precipitated at the very beginning of decomposition and worked as heterogeneous nuclei for L1{sub 2}-Al{sub 3}Zr with spherical morphology after being aged at 400 °C for 2 h. Quasi-static coarsening happened as the aging treatment lasted from 2 h to 200 h. However, distribution of Zr and Y atoms in Al{sub 3}(Zr,Y) is nearly uniform and Al{submore » 3}(Zr,Y) do not have the typical “Al{sub 3}RE core-Al{sub 3}Zr shell” structure which observed in other RE containing Al-Zr-RE alloys with L1{sub 2}-Al{sub 3}RE as nuclei. First principles calculations revealed that binding energy between Y and Zr is strong during the growth of Al{sub 3}(Zr,Y), which led to the co-precipitation of Y and Zr atoms and attribute to the evolution of Al{sub 3}(Zr,Y). - Highlights: •Al{sub 3}Y precipitated firstly and then became nuclei for Al{sub 3}Zr during aging of Al-Zr-Y. •Al{sub 3}(Zr,Y) precipitates do not have the typical “Al{sub 3}Y core-Al{sub 3}Zr shell” structure. •Strong binding between Y and Zr led to the co-precipitation of Y and Zr atoms.« less

  2. Multipolar electrostatics for proteins: atom-atom electrostatic energies in crambin.

    PubMed

    Yuan, Yongna; Mills, Matthew J L; Popelier, Paul L A

    2014-02-15

    Accurate electrostatics necessitates the use of multipole moments centered on nuclei or extra point charges centered away from the nuclei. Here, we follow the former alternative and investigate the convergence behavior of atom-atom electrostatic interactions in the pilot protein crambin. Amino acids are cut out from a Protein Data Bank structure of crambin, as single amino acids, di, or tripeptides, and are then capped with a peptide bond at each side. The atoms in the amino acids are defined through Quantum Chemical Topology (QCT) as finite volume electron density fragments. Atom-atom electrostatic energies are computed by means of a multipole expansion with regular spherical harmonics, up to a total interaction rank of L = ℓA+ ℓB + 1 = 10. The minimum internuclear distance in the convergent region of all the 15 possible types of atom-atom interactions in crambin that were calculated based on single amino acids are close to the values calculated from di and tripeptides. Values obtained at B3LYP/aug-cc-pVTZ and MP2/aug-cc-pVTZ levels are only slightly larger than those calculated at HF/6-31G(d,p) level. This convergence behavior is transferable to the well-known amyloid beta polypeptide Aβ1-42. Moreover, for a selected central atom, the influence of its neighbors on its multipole moments is investigated, and how far away this influence can be ignored is also determined. Finally, the convergence behavior of AMBER becomes closer to that of QCT with increasing internuclear distance. Copyright © 2013 Wiley Periodicals, Inc.

  3. Improved limit on the Ra 225 electric dipole moment

    DOE PAGES

    Bishof, Michael; Parker, Richard H.; Bailey, Kevin G.; ...

    2016-08-03

    In this study, octupole-deformed nuclei, such as that of 225Ra, are expected to amplify observable atomic electric dipole moments (EDMs) that arise from time-reversal and parity-violating interactions in the nuclear medium. In 2015 we reported the first “proof-of-principle” measurement of the 225Ra atomic EDM.

  4. Improved limit on the Ra 225 electric dipole moment

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Bishof, Michael; Parker, Richard H.; Bailey, Kevin G.

    In this study, octupole-deformed nuclei, such as that of 225Ra, are expected to amplify observable atomic electric dipole moments (EDMs) that arise from time-reversal and parity-violating interactions in the nuclear medium. In 2015 we reported the first “proof-of-principle” measurement of the 225Ra atomic EDM.

  5. E1 transitions from octupole vibration states

    NASA Astrophysics Data System (ADS)

    Cottle, P. D.

    1993-04-01

    Electric dipole moments are extracted from data for E1 transitions deexciting octupole vibration states in nineteen nuclei. The moments are then compared to values calculated using the droplet model prescription of Dorso, Myers, and Swiatecki. It is found that the E1 moments in quadrupole deformed nuclei can be reproduced with the droplet model using the same model parameters that reproduce atomic masses and fission barriers. This result supports the suggestion of Butler and Nazarewicz that single particle effects are usually much smaller than macroscopic effects in E1 transitions associated with octupole vibrations in reflection symmetric deformed nuclei.

  6. Nucleon Isovector Pairing in Nuclei: Microscopic Approach, Boson Representation, and Collective Model

    NASA Astrophysics Data System (ADS)

    Jolos, R. V.; Kartavenko, V. G.; Kolganova, E. A.

    2018-03-01

    Nucleon pair correlations in atomic nuclei are analyzed within a nuclear microscopic model with residual isovector pairing forces. These are formulated in the boson representation of fermion operators whereby the collective mode of pair excitations can be isolated without restricting the size of the one-particle basis. This method allows one to analyze the fluctuations in the nonsuperfluid phase of nuclear matter, its phase transition to the superfluid phase, and strong pair correlations. The performance of the method is exemplified by numerical results for the nuclei in the vicinity of the doubly magic 56Ni nucleus.

  7. Momentum sharing in imbalanced Fermi systems

    NASA Astrophysics Data System (ADS)

    Hen, O.; Sargsian, M.; Weinstein, L. B.; Piasetzky, E.; Hakobyan, H.; Higinbotham, D. W.; Braverman, M.; Brooks, W. K.; Gilad, S.; Adhikari, K. P.; Arrington, J.; Asryan, G.; Avakian, H.; Ball, J.; Baltzell, N. A.; Battaglieri, M.; Beck, A.; Beck, S. May-Tal; Bedlinskiy, I.; Bertozzi, W.; Biselli, A.; Burkert, V. D.; Cao, T.; Carman, D. S.; Celentano, A.; Chandavar, S.; Colaneri, L.; Cole, P. L.; Crede, V.; D'Angelo, A.; De Vita, R.; Deur, A.; Djalali, C.; Doughty, D.; Dugger, M.; Dupre, R.; Egiyan, H.; El Alaoui, A.; El Fassi, L.; Elouadrhiri, L.; Fedotov, G.; Fegan, S.; Forest, T.; Garillon, B.; Garcon, M.; Gevorgyan, N.; Ghandilyan, Y.; Gilfoyle, G. P.; Girod, F. X.; Goetz, J. T.; Gothe, R. W.; Griffioen, K. A.; Guidal, M.; Guo, L.; Hafidi, K.; Hanretty, C.; Hattawy, M.; Hicks, K.; Holtrop, M.; Hyde, C. E.; Ilieva, Y.; Ireland, D. G.; Ishkanov, B. I.; Isupov, E. L.; Jiang, H.; Jo, H. S.; Joo, K.; Keller, D.; Khandaker, M.; Kim, A.; Kim, W.; Klein, F. J.; Koirala, S.; Korover, I.; Kuhn, S. E.; Kubarovsky, V.; Lenisa, P.; Levine, W. I.; Livingston, K.; Lowry, M.; Lu, H. Y.; MacGregor, I. J. D.; Markov, N.; Mayer, M.; McKinnon, B.; Mineeva, T.; Mokeev, V.; Movsisyan, A.; Camacho, C. Munoz; Mustapha, B.; Nadel-Turonski, P.; Niccolai, S.; Niculescu, G.; Niculescu, I.; Osipenko, M.; Pappalardo, L. L.; Paremuzyan, R.; Park, K.; Pasyuk, E.; Phelps, W.; Pisano, S.; Pogorelko, O.; Price, J. W.; Procureur, S.; Prok, Y.; Protopopescu, D.; Puckett, A. J. R.; Rimal, D.; Ripani, M.; Ritchie, B. G.; Rizzo, A.; Rosner, G.; Roy, P.; Rossi, P.; Sabatié, F.; Schott, D.; Schumacher, R. A.; Sharabian, Y. G.; Smith, G. D.; Shneor, R.; Sokhan, D.; Stepanyan, S. S.; Stepanyan, S.; Stoler, P.; Strauch, S.; Sytnik, V.; Taiuti, M.; Tkachenko, S.; Ungaro, M.; Vlassov, A. V.; Voutier, E.; Walford, N. K.; Wei, X.; Wood, M. H.; Wood, S. A.; Zachariou, N.; Zana, L.; Zhao, Z. W.; Zheng, X.; Zonta, I.; aff16

    2014-10-01

    The atomic nucleus is composed of two different kinds of fermions: protons and neutrons. If the protons and neutrons did not interact, the Pauli exclusion principle would force the majority of fermions (usually neutrons) to have a higher average momentum. Our high-energy electron-scattering measurements using 12C, 27Al, 56Fe, and 208Pb targets show that even in heavy, neutron-rich nuclei, short-range interactions between the fermions form correlated high-momentum neutron-proton pairs. Thus, in neutron-rich nuclei, protons have a greater probability than neutrons to have momentum greater than the Fermi momentum. This finding has implications ranging from nuclear few-body systems to neutron stars and may also be observable experimentally in two-spin-state, ultracold atomic gas systems.

  8. Are there any narrow K--nuclear states?

    NASA Astrophysics Data System (ADS)

    Hrtánková, Jaroslava; Mareš, Jiří

    2017-07-01

    We performed self-consistent calculations of K--nuclear quasi-bound states using a single-nucleon K- optical potential derived from chiral meson-baryon coupled-channel interaction models, supplemented by a phenomenological K- multinucleon potential introduced recently to achieve good fits to kaonic atom data [1]. Our calculations show that the effect of K- multinucleon interactions on K- widths in nuclei is decisive. The resulting widths are considerably larger than corresponding binding energies. Moreover, when the density dependence of the K--multinucleon interactions derived in the fits of kaonic atoms is extended to the nuclear interior, the only two models acceptable after imposing as additional constraint the single-nucleon fraction of K- absorption at rest do not yield any kaonic nuclear bound state in majority of considered nuclei.

  9. Effects of rotation of fissioning nuclei in the angular distributions of prompt neutrons and gamma rays originating from the polarized-neutron-induced fission of 233U and 235U nuclei

    NASA Astrophysics Data System (ADS)

    Danilyan, G. V.; Klenke, J.; Kopach, Yu. N.; Krakhotin, V. A.; Novitsky, V. V.; Pavlov, V. S.; Shatalov, P. B.

    2014-06-01

    The results of an experiment devoted to searches for effects of rotation of fissioning nuclei in the angular distributions of prompt neutrons and gamma rays originating from the polarized-neutron-induced fission of 233U nuclei are presented. The effects discovered in these angular distributions are opposite in sign to their counterparts in the polarized-neutron-induced fission of 235U nuclei. This is at odds with data on the relative signs of respective effects in the angular distribution of alpha particles from the ternary fission of the same nuclei and may be indicative of problems in the model currently used to describe the effect in question. The report on which this article is based was presented at the seminar held at the Institute of Theoretical and Experimental Physics and dedicated to the 90th anniversary of the birth of Yu.G. Abov, corresponding member of Russian Academy of Sciences, Editor in Chief of the journal Physics of Atomic Nuclei.

  10. Excitation of Nuclei and Atoms Trapping in Optical Fields of High Intensity

    DTIC Science & Technology

    2006-11-01

    the new relativistic wave equation for half- spin particle interacting with the electromagnetic field. The proposed equation is Lorentz and gauge ...CONTENTS Task 1. Gamma-ray laser with hidden inversion of nuclear state populations 3 Introduction 3 Recoil-accompanied nuclear...31 Task 2. Extended ensemble of monoenergetic atoms 33 Introduction 33 Results 37 Conclusion 66

  11. Magnesium and Calcium in Isolated Cell Nuclei

    PubMed Central

    Naora, H.; Naora, H.; Mirsky, A. E.; Allfrey, V. G.

    1961-01-01

    The calcium and magnesium contents of thymus nuclei have been determined and the nuclear sites of attachment of these two elements have been studied. The nuclei used for these purposes were isolated in non-aqueous media and in sucrose solutions. Non-aqueous nuclei contain 0.024 per cent calcium and 0.115 per cent magnesium. Calcium and magnesium are held at different sites. The greater part of the magnesium is bound to DNA, probably to its phosphate groups. Evidence is presented that the magnesium atoms combined with the phosphate groups of DNA are also attached to mononucleotides. There is reason to believe that those DNA-phosphate groups to which magnesium is bound, less than 1/10th of the total, are metabolically active, while those to which histones are attached seem to be inactive. PMID:13727745

  12. Unraveling Metal-insulator Transition Mechanism of VO2 Triggered by Tungsten Doping

    PubMed Central

    Tan, Xiaogang; Yao, Tao; Long, Ran; Sun, Zhihu; Feng, Yajuan; Cheng, Hao; Yuan, Xun; Zhang, Wenqing; Liu, Qinghua; Wu, Changzheng; Xie, Yi; Wei, Shiqiang

    2012-01-01

    Understanding the mechanism of W-doping induced reduction of critical temperature (TC) for VO2 metal-insulator transition (MIT) is crucial for both fundamental study and technological application. Here, using synchrotron radiation X-ray absorption spectroscopy combined with first-principles calculations, we unveil the atomic structure evolutions of W dopant and its role in tailoring the TC of VO2 MIT. We find that the local structure around W atom is intrinsically symmetric with a tetragonal-like structure, exhibiting a concentration-dependent evolution involving the initial distortion, further repulsion, and final stabilization due to the strong interaction between doped W atoms and VO2 lattices across the MIT. These results directly give the experimental evidence that the symmetric W core drives the detwisting of the nearby asymmetric monoclinic VO2 lattice to form rutile-like VO2 nuclei, and the propagations of these W-encampassed nuclei through the matrix lower the thermal energy barrier for phase transition. PMID:22737402

  13. Helium vs. Proton Induced Displacement Damage in Electronic Materials

    NASA Technical Reports Server (NTRS)

    Ringo, Sawnese; Barghouty, A. F.

    2010-01-01

    In this project, the specific effects of displacement damage due to the passage of protons and helium nuclei on some typical electronic materials will be evaluated and contrasted. As the electronic material absorbs the energetic proton and helium momentum, degradation of performance occurs, eventually leading to overall failure. Helium nuclei traveling at the same speed as protons are expected to impart more to the material displacement damage; due to the larger mass, and thus momentum, of helium nuclei compared to protons. Damage due to displacement of atoms in their crystalline structure can change the physical properties and hence performance of the electronic materials.

  14. High resolution gamma-ray spectroscopy and the fascinating angular momentum realm of the atomic nucleus

    NASA Astrophysics Data System (ADS)

    Riley, M. A.; Simpson, J.; Paul, E. S.

    2016-12-01

    In 1974 Aage Bohr and Ben Mottelson predicted the different ‘phases’ that may be expected in deformed nuclei as a function of increasing angular momentum and excitation energy all the way up to the fission limit. While admitting their picture was highly conjectural they confidently stated ‘...with the ingenious experimental approaches that are being developed, we may look forward with excitement to the detailed spectroscopic studies that will illuminate the behaviour of the spinning quantised nucleus’. High resolution gamma-ray spectroscopy has indeed been a major tool in studying the structure of atomic nuclei and has witnessed numerous significant advances over the last four decades. This article will select highlights from investigations at the Niels Bohr Institute, Denmark, and Daresbury Laboratory, UK, in the late 1970s and early 1980s, some of which have continued at other national laboratories in Europe and the USA to the present day. These studies illustrate the remarkable diversity of phenomena and symmetries exhibited by nuclei in the angular momentum-excitation energy plane that continue to surprise and fascinate scientists.

  15. Momentum sharing in imbalanced Fermi systems

    DOE PAGES

    Hen, O.; Sargsian, M.; Weinstein, L. B.; ...

    2014-10-16

    The atomic nucleus is composed of two different kinds of fermions, protons and neutrons. If the protons and neutrons did not interact, the Pauli exclusion principle would force the majority fermions (usually neutrons) to have a higher average momentum. Our high-energy electron scattering measurements using 12C, 27Al, 56Fe and 208Pb targets show that, even in heavy neutron-rich nuclei, short-range interactions between the fermions form correlated high-momentum neutron-proton pairs. Thus, in neutron-rich nuclei, protons have a greater probability than neutrons to have momentum greater than the Fermi momentum. This finding has implications ranging from nuclear few body systems to neutron starsmore » and may also be observable experimentally in two-spin state, ultra-cold atomic gas systems.« less

  16. Nuclear physics. Momentum sharing in imbalanced Fermi systems.

    PubMed

    Hen, O; Sargsian, M; Weinstein, L B; Piasetzky, E; Hakobyan, H; Higinbotham, D W; Braverman, M; Brooks, W K; Gilad, S; Adhikari, K P; Arrington, J; Asryan, G; Avakian, H; Ball, J; Baltzell, N A; Battaglieri, M; Beck, A; May-Tal Beck, S; Bedlinskiy, I; Bertozzi, W; Biselli, A; Burkert, V D; Cao, T; Carman, D S; Celentano, A; Chandavar, S; Colaneri, L; Cole, P L; Crede, V; D'Angelo, A; De Vita, R; Deur, A; Djalali, C; Doughty, D; Dugger, M; Dupre, R; Egiyan, H; El Alaoui, A; El Fassi, L; Elouadrhiri, L; Fedotov, G; Fegan, S; Forest, T; Garillon, B; Garcon, M; Gevorgyan, N; Ghandilyan, Y; Gilfoyle, G P; Girod, F X; Goetz, J T; Gothe, R W; Griffioen, K A; Guidal, M; Guo, L; Hafidi, K; Hanretty, C; Hattawy, M; Hicks, K; Holtrop, M; Hyde, C E; Ilieva, Y; Ireland, D G; Ishkanov, B I; Isupov, E L; Jiang, H; Jo, H S; Joo, K; Keller, D; Khandaker, M; Kim, A; Kim, W; Klein, F J; Koirala, S; Korover, I; Kuhn, S E; Kubarovsky, V; Lenisa, P; Levine, W I; Livingston, K; Lowry, M; Lu, H Y; MacGregor, I J D; Markov, N; Mayer, M; McKinnon, B; Mineeva, T; Mokeev, V; Movsisyan, A; Munoz Camacho, C; Mustapha, B; Nadel-Turonski, P; Niccolai, S; Niculescu, G; Niculescu, I; Osipenko, M; Pappalardo, L L; Paremuzyan, R; Park, K; Pasyuk, E; Phelps, W; Pisano, S; Pogorelko, O; Price, J W; Procureur, S; Prok, Y; Protopopescu, D; Puckett, A J R; Rimal, D; Ripani, M; Ritchie, B G; Rizzo, A; Rosner, G; Roy, P; Rossi, P; Sabatié, F; Schott, D; Schumacher, R A; Sharabian, Y G; Smith, G D; Shneor, R; Sokhan, D; Stepanyan, S S; Stepanyan, S; Stoler, P; Strauch, S; Sytnik, V; Taiuti, M; Tkachenko, S; Ungaro, M; Vlassov, A V; Voutier, E; Walford, N K; Wei, X; Wood, M H; Wood, S A; Zachariou, N; Zana, L; Zhao, Z W; Zheng, X; Zonta, I

    2014-10-31

    The atomic nucleus is composed of two different kinds of fermions: protons and neutrons. If the protons and neutrons did not interact, the Pauli exclusion principle would force the majority of fermions (usually neutrons) to have a higher average momentum. Our high-energy electron-scattering measurements using (12)C, (27)Al, (56)Fe, and (208)Pb targets show that even in heavy, neutron-rich nuclei, short-range interactions between the fermions form correlated high-momentum neutron-proton pairs. Thus, in neutron-rich nuclei, protons have a greater probability than neutrons to have momentum greater than the Fermi momentum. This finding has implications ranging from nuclear few-body systems to neutron stars and may also be observable experimentally in two-spin-state, ultracold atomic gas systems. Copyright © 2014, American Association for the Advancement of Science.

  17. Method of controlling fusion reaction rates

    DOEpatents

    Kulsrud, Russell M.; Furth, Harold P.; Valeo, Ernest J.; Goldhaber, Maurice

    1988-01-01

    A method of controlling the reaction rates of the fuel atoms in a fusion reactor comprises the step of polarizing the nuclei of the fuel atoms in a particular direction relative to the plasma confining magnetic field. Fusion reaction rates can be increased or decreased, and the direction of emission of the reaction products can be controlled, depending on the choice of polarization direction.

  18. Nuclear Stability and Nucleon-Nucleon Interactions in Introductory and General Chemistry Textbooks

    ERIC Educational Resources Information Center

    Millevolte, Anthony

    2010-01-01

    The nucleus is a highly dense and highly charged substructure of atoms. In the nuclei of all atoms beyond hydrogen, multiple protons are in close proximity to each other in spite of strong electrostatic repulsions between them. The attractive internucleon strong force is described and its origin explained by using a simple quark model for the…

  19. Method of controlling fusion reaction rates

    DOEpatents

    Kulsrud, Russell M.; Furth, Harold P.; Valeo, Ernest J.; Goldhaber, Maurice

    1988-03-01

    A method of controlling the reaction rates of the fuel atoms in a fusion reactor comprises the step of polarizing the nuclei of the fuel atoms in a particular direction relative to the plasma confining magnetic field. Fusion reaction rates can be increased or decreased, and the direction of emission of the reaction products can be controlled, depending on the choice of polarization direction.

  20. And so Ad Infinitum: The Search for Quark and Lepton Substructure

    ERIC Educational Resources Information Center

    Lincoln, Don

    2018-01-01

    The saga of the search for the ultimate constituents of matter has long been one of finding a seemingly fundamental structure that, in turn, was found to be made of even smaller building blocks. Matter is made of molecules. Molecules are in turn made of atoms, which are themselves made of electrons and atomic nuclei. The nucleus consists of…

  1. Magnitude of finite-nucleus-size effects in relativistic density functional computations of indirect NMR nuclear spin-spin coupling constants.

    PubMed

    Autschbach, Jochen

    2009-09-14

    A spherical Gaussian nuclear charge distribution model has been implemented for spin-free (scalar) and two-component (spin-orbit) relativistic density functional calculations of indirect NMR nuclear spin-spin coupling (J-coupling) constants. The finite nuclear volume effects on the hyperfine integrals are quite pronounced and as a consequence they noticeably alter coupling constants involving heavy NMR nuclei such as W, Pt, Hg, Tl, and Pb. Typically, the isotropic J-couplings are reduced in magnitude by about 10 to 15 % for couplings between one of the heaviest NMR nuclei and a light atomic ligand, and even more so for couplings between two heavy atoms. For a subset of the systems studied, viz. the Hg atom, Hg(2) (2+), and Tl--X where X=Br, I, the basis set convergence of the hyperfine integrals and the coupling constants was monitored. For the Hg atom, numerical and basis set calculations of the electron density and the 1s and 6s orbital hyperfine integrals are directly compared. The coupling anisotropies of TlBr and TlI increase by about 2 % due to finite-nucleus effects.

  2. Study to perform preliminary experiments to evaluate particle generation and characterization techniques for zero-gravity cloud physics experiments

    NASA Technical Reports Server (NTRS)

    Katz, U.

    1982-01-01

    Methods of particle generation and characterization with regard to their applicability for experiments requiring cloud condensation nuclei (CCN) of specified properties were investigated. Since aerosol characterization is a prerequisite to assessing performance of particle generation equipment, techniques for characterizing aerosol were evaluated. Aerosol generation is discussed, and atomizer and photolytic generators including preparation of hydrosols (used with atomizers) and the evaluation of a flight version of an atomizer are studied.

  3. alpha-decay half-lives and Q{sub a}lpha values of superheavy nuclei

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dong Jianmin; Graduate University of Chinese Academy of Sciences, Beijing 100049; School of Nuclear Science and Technology, Lanzhou University, Lanzhou 730000

    2010-06-15

    The alpha-decay half-lives of recently synthesized superheavy nuclei (SHN) are investigated by employing a unified fission model (UFM) where a new method to calculate the assault frequency of alpha emission is used. The excellent agreement with the experimental data indicates the UFM is a useful tool to investigate these alpha decays. It is found that the alpha-decay half-lives become more and more insensitive to the Q{sub a}lpha values as the atomic number increases on the whole, which is favorable for us to predict the half-lives of SHN. In addition, a formula is proposed to compute the Q{sub a}lpha values formore » the nuclei with Z>=92 and N>=140 with a good accuracy, according to which the long-lived SHN should be neutron rich. Several weeks ago, two isotopes of a new element with atomic number Z=117 were synthesized and their alpha-decay chains have been observed. The Q{sub a}lpha formula is found to work well for these nuclei, confirming its predictive power. The experimental half-lives are well reproduced by employing the UFM with the experimental Q{sub a}lpha values. This fact that the experimental half-lives are compatible with experimental Q{sub a}lpha values supports the synthesis of a new element 117 and the experimental measurements to a certain extent.« less

  4. New dimensions of the periodic system: superheavy, superneutronic, superstrange, antimatter nuclei

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Greiner, Walter

    2010-12-23

    The possibilities for the extension of the periodic system into the islands of superheavy (SH) elements, to and beyond the neutron drip line and to the sectors of strangeness and antimatter are discussed. The multi-nucleon transfer processes in low-energy damped collisions of heavy actinide nuclei may help us to fill the gap between the nuclei produced in the ''hot'' fusion reactions and the continent of known nuclei. In these reactions we may also investigate the ''island of stability''. In many such collisions the lifetime of the composite giant system consisting of two touching nuclei turns out to be rather longmore » ({>=}10{sup -20} s); sufficient for observing line structure in spontaneous positron emission from super-strong electric fields (vacuum decay), a fundamental QED process not observed yet experimentally. At the neutron-rich sector near the drip line islands and extended ridges of quasistable nuclei are predicted by HF calculations. Such nuclei, as well as very long living superheavy nuclei may be provided in double atomic bomb explosions. A tremendously rich scenario of new nuclear structure emerges with new magic numbers in the strangeness domain. Various production mechanisms are discussed for these objects and for antinuclei in high energy heavy-ion collisions.« less

  5. Non-classical nuclei and growth kinetics of Cr precipitates in FeCr alloys during ageing

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Li, Yulan; Hu, Shenyang Y.; Zhang, Lei

    2014-01-10

    In this manuscript, we quantitatively calculated the thermodynamic properties of critical nuclei of Cr precipitates in FeCr alloys. The concentration profiles of the critical nuclei and nucleation energy barriers were predicted by the constrained shrinking dimer dynamics (CSDD) method. It is found that Cr concentration distribution in the critical nuclei strongly depend on the overall Cr concentration as well as temperature. The critical nuclei are non-classical because the concentration in the nuclei is smaller than the thermodynamic equilibrium value. These results are in agreement with atomic probe observation. The growth kinetics of both classical and non-classical nuclei was investigated bymore » the phase field approach. The simulations of critical nucleus evolution showed a number of interesting phenomena: 1) a critical classical nucleus first shrinks toward its non-classical nucleus and then grows; 2) a non-classical nucleus has much slower growth kinetics at its earlier growth stage compared to the diffusion-controlled growth kinetics. 3) a critical classical nucleus grows faster at the earlier growth stage than the non-classical nucleus. All of these results demonstrate that it is critical to introduce the correct critical nuclei in order to correctly capture the kinetics of precipitation.« less

  6. Double binding energy differences: Mean-field or pairing effect?

    NASA Astrophysics Data System (ADS)

    Qi, Chong

    2012-10-01

    In this Letter we present a systematic analysis on the average interaction between the last protons and neutrons in atomic nuclei, which can be extracted from the double differences of nuclear binding energies. The empirical average proton-neutron interaction Vpn thus derived from experimental data can be described in a very simple form as the interplay of the nuclear mean field and the pairing interaction. It is found that the smooth behavior as well as the local fluctuations of the Vpn in even-even nuclei with N ≠ Z are dominated by the contribution from the proton-neutron monopole interactions. A strong additional contribution from the isoscalar monopole interaction and isovector proton-neutron pairing interaction is seen in the Vpn for even-even N = Z nuclei and for the adjacent odd-A nuclei with one neutron or proton being subtracted.

  7. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Gupta, J. B.; Hamilton, J. H.

    The change in the structure of the collective levels with spin angular momentum in atomic nuclei is often expressed in terms of the classical concepts of the kinematic and the dynamic moments of inertia varying with spin. For the well deformed even-even nuclei the kinematic moment of inertia increases with spin up to 10%-20%, at say I{sup {pi}} = 12{sup +}. However, for the shape transitional nuclei, or almost spherical nuclei, it increases with spin much faster. The pitfalls of using the rotor model form of kinematic moment of inertia in such cases are pointed out here. Alternative methods ofmore » extracting the nuclear structure information are explored. The important role of the ground state deformation is illustrated. The use of the power index formula for evaluating the effective moment of inertia, free from the assumption of the rotor model, is described.« less

  8. Gd(III) complexes as paramagnetic tags: Evaluation of the spin delocalization over the nuclei of the ligand

    NASA Astrophysics Data System (ADS)

    Collauto, A.; Feintuch, A.; Qi, M.; Godt, A.; Meade, T.; Goldfarb, D.

    2016-02-01

    Complexes of the Gd(III) ion are currently being established as spin labels for distance determination in biomolecules by pulse dipolar spectroscopy. Because Gd(III) is an f ion, one expects electron spin density to be localized on the Gd(III) ion - an important feature for the mentioned application. Most of the complex ligands have nitrogens as Gd(III) coordinating atoms. Therefore, measurement of the 14N hyperfine coupling gives access to information on the localization of the electron spin on the Gd(III) ion. We carried out W-band, 1D and 2D 14N and 1H ENDOR measurements on the Gd(III) complexes Gd-DOTA, Gd-538, Gd-595, and Gd-PyMTA that serve as spin labels for Gd-Gd distance measurements. The obtained 14N spectra are particularly well resolved, revealing both the hyperfine and nuclear quadrupole splittings, which were assigned using 2D Mims ENDOR experiments. Additionally, the spectral contributions of the two different types of nitrogen atoms of Gd-PyMTA, the aliphatic N atom and the pyridine N atom, were distinguishable. The 14N hyperfine interaction was found to have a very small isotropic hyperfine component of -0.25 to -0.37 MHz. Furthermore, the anisotropic hyperfine interactions with the 14N nuclei and with the non-exchangeable protons of the ligands are well described by the point-dipole approximation using distances derived from the crystal structures. We therefore conclude that the spin density is fully localized on the Gd(III) ion and that the spin density distribution over the nuclei of the ligands is rightfully ignored when analyzing distance measurements.

  9. Electric field imaging of single atoms

    PubMed Central

    Shibata, Naoya; Seki, Takehito; Sánchez-Santolino, Gabriel; Findlay, Scott D.; Kohno, Yuji; Matsumoto, Takao; Ishikawa, Ryo; Ikuhara, Yuichi

    2017-01-01

    In scanning transmission electron microscopy (STEM), single atoms can be imaged by detecting electrons scattered through high angles using post-specimen, annular-type detectors. Recently, it has been shown that the atomic-scale electric field of both the positive atomic nuclei and the surrounding negative electrons within crystalline materials can be probed by atomic-resolution differential phase contrast STEM. Here we demonstrate the real-space imaging of the (projected) atomic electric field distribution inside single Au atoms, using sub-Å spatial resolution STEM combined with a high-speed segmented detector. We directly visualize that the electric field distribution (blurred by the sub-Å size electron probe) drastically changes within the single Au atom in a shape that relates to the spatial variation of total charge density within the atom. Atomic-resolution electric field mapping with single-atom sensitivity enables us to examine their detailed internal and boundary structures. PMID:28555629

  10. Relativistic Spin-Orbit Heavy Atom on the Light Atom NMR Chemical Shifts: General Trends Across the Periodic Table Explained.

    PubMed

    Vícha, Jan; Komorovsky, Stanislav; Repisky, Michal; Marek, Radek; Straka, Michal

    2018-06-12

    The importance of relativistic effects on the NMR parameters in heavy-atom (HA) compounds, particularly the SO-HALA (Spin-Orbit Heavy Atom on the Light Atom) effect on NMR chemical shifts, has been known for about 40 years. Yet, a general correlation between the electronic structure and SO-HALA effect has been missing. By analyzing 1 H NMR chemical shifts of the sixth-period hydrides (Cs-At), we discovered general electronic-structure principles and mechanisms that dictate the size and sign of the SO-HALA NMR chemical shifts. In brief, partially occupied HA valence shells induce relativistic shielding at the light atom (LA) nuclei, while empty HA valence shells induce relativistic deshielding. In particular, the LA nucleus is relativistically shielded in 5d 2 -5d 8 and 6p 4 HA hydrides and deshielded in 4f 0 , 5d 0 , 6s 0 , and 6p 0 HA hydrides. This general and intuitive concept explains periodic trends in the 1 H NMR chemical shifts along the sixth-period hydrides (Cs-At) studied in this work. We present substantial evidence that the introduced principles have a general validity across the periodic table and can be extended to nonhydride LAs. The decades-old question of why compounds with occupied frontier π molecular orbitals (MOs) cause SO-HALA shielding at the LA nuclei, while the frontier σ MOs cause deshielding is answered. We further derive connection between the SO-HALA NMR chemical shifts and Spin-Orbit-induced Electron Deformation Density (SO-EDD), a property that can be obtained easily from differential electron densities and can be represented graphically. SO-EDD provides an intuitive understanding of the SO-HALA effect in terms of the depletion/concentration of the electron density at LA nuclei caused by spin-orbit coupling due to HA in the presence of a magnetic field. Using an analogy between the SO-EDD concept and arguments from classic NMR theory, the complex question of the SO-HALA NMR chemical shifts becomes easily understandable for a wide chemical audience.

  11. A UHV compatible source for a highly polarized thermal atomic beam of radioactive 8Li

    NASA Astrophysics Data System (ADS)

    Jänsch, H. J.; Kirchner, G.; Kühlert, O.; Lisowski, M.; Paggel, J. J.; Platzer, R.; Schillinger, R.; Tilsner, H.; Weindel, C.; Winnefeld, H.; Fick, D.

    2000-12-01

    A beam of the radioactive isotope 8Li is prepared at thermal velocities. The nuclei are highly spin polarized by transverse optical pumping of the thermal beam. The installation is ultra-high vacuum (UHV) compatible in a non-UHV accelerator environment. Since the atomic beam is used in a surface science experiment, where contamination must be avoided, special emphasis is given to the vacuum coupling of the accelerator/ 8Li production/surface experimental areas. The atomic beam is produced by stopping the nuclear reaction products and evaporating them again from high-temperature graphite. To enhance the atomic beam, a novel tubular thermalizer is applied. The thermal polarized atomic beam intensity is approximately 5×10 8 atoms/s sr.

  12. Is Einstein the Father of the Atomic Bomb

    NASA Astrophysics Data System (ADS)

    Lustig, Harry

    2009-05-01

    Soon after the American atomic bombs were dropped on Hiroshima and Nagasaki, the notion took hold in the popular mind that Albert Einstein was ``the father of the bomb.'' The claim of paternity rests on the belief that E=mc2 is what makes the release of enormous amounts of energy in the fission process possible and that the atomic bomb could not have been built without it. This is a misapprehension. Most physicists have known that all along. Nevertheless in his reaction to the opera Dr. Atomic, a prominent physicist claimed that Einstein's discovery that matter can be transformed into energy ``is precisely what made the bomb possible.'' In fact what makes the fission reaction and one of its applications,the atomic bomb, possible is the smaller binding energies of fission products compared to the binding energies of the nuclei that undergo fission.The binding energies of nuclei are a well understood consequence of the numbers and arrangements of protons and neutrons in the nucleus and of quantum-mechanical effects. The realization that composite systems have binding energies predates relativity. In the 19th century they were ascribed to potential and other forms of energy that reside in the system. With Einstein they became rest mass energy. While E=mc2 is not the cause of fission, measuring the masses of the participants in the reaction does permit an easy calculation of the kinetic energy that is released.

  13. Feshbach Prize: New Phenomena and New Physics from Strongly-Correlated Quantum Matter

    NASA Astrophysics Data System (ADS)

    Carlson, Joseph A.

    2017-01-01

    Strongly correlated quantum matter is ubiquitous in physics from cold atoms to nuclei to the cold dense matter found in neutron stars. Experiments from table-top to the extremely large scale experiments including FRIB and LIGO will help determine the properties of matter across an incredible scale of distances and energies. Questions to be addressed include the existence of exotic states of matter in cold atoms and nuclei, the response of this correlated matter to external probes, and the behavior of matter in extreme astrophysical environments. A more complete understanding is required, both to understand these diverse phenomena and to employ this understanding to probe for new underlying physics in experiments including neutrinoless double beta decay and accelerator neutrino experiments. I will summarize some aspects of our present understanding and highlight several important prospects for the future.

  14. Preface

    NASA Astrophysics Data System (ADS)

    Kowalska, Magdalena; Błaszczak, Zdzislaw

    2017-11-01

    It is with great pleasure that we are presenting the subsequent volume of the International Poznan Workshop proceedings. The conferences of this cycle have been since the beginning devoted to laser light interaction with atomic nuclei and since more recently also to the applications of ion-storage devices. The first edition entitled "Laser Spectroscopy of Atomic Nuclei" took place in Dubna in December 1990, and since then the subsequent conferences have been held every two to three years in Poznan, where they have been jointly organized by the Faculty of Physics at the Adam Mickiewicz University (Poznan) and the Flerov Laboratory of Nuclear Reactions at the Joint Institute of Nuclear Research (Dubna). The conferences have enjoyed increasing popularity and have attracted increasing numbers of specialists from a number of research institutions engaged in laser spectroscopy of radioactive and other exotic (e.g. anti-) atomic nuclei and related instruments. Over the years the workshops have gained a reputation of presenting research of a high scientific level and having impact on the directions of future studies. The 2016 workshop on the Application of Lasers and Storage Devices in Atomic Nuclei Research has been already the 10th edition and it was a pleasure to see that the event was thriving and the participants were enjoying it in all fronts. Around 100 scientists met on May 16 -19 in Poznan for the 4-day event. They were even more international than in the previous edition, representing institutes in Europe, North America, Japan, and even Australia. Many have returned to Poznan, but there were also new faces, especially among the younger participants. It was great to see the leaders in their topics discussing physics, but not only, with PhD students and starting post-docs. More than sixty talks were delivered, reflecting well the state-of-the art in the covered fields which were all related to the techniques, experimental results and theory connected to lasers and storage devices applied to exotic nuclei. The presentations were supplemented with many posters covering even more results. We hope that the participants also enjoyed the concert of renaissance music. In this warm atmosphere (much warmer than the temperatures outside the lecture hall), we are looking forward to the 11 th edition, which has been already announced to take place again in Poznan. In the next 3 years many new results will be certainly collected, so that without doubt we will participate in another interesting workshop.

  15. All the observed universe has contributed to life.

    PubMed

    Davies, R E; Koch, R H

    1991-12-30

    This paper presents evidence that virtually all electrons and nuclei of the atoms that are or have been part of living matter on Earth came from almost all stars in our and nearby galaxies and even from all other galaxies in the Universe that have produced observed high-energy gamma rays. However, a standard 70 kg human is always making about 7 3He, 600 40Ca, and 3000 14N nuclei every second by radioactive decay of 3H, 40K, and 14C, respectively.

  16. ORBITING CLUSTERS IN ATOMIC NUCLEI

    PubMed Central

    Pauling, Linus

    1969-01-01

    As an alternative to their description as vibrational levels, the low excited states of even-even nuclei can be described as rotational states of a helion, dineutron, diproton, or other cluster about the rest of the nucleus, leading to reasonable values of the average distance between centers of the clusters. Some states involve rotational excitation of two or more helions or other clusters. The nature of the rotating clusters is determined by the relation of the neutron and proton numbers to the magic numbers. PMID:16591799

  17. Unusual chemical compositions of noctilucent-cloud particle nuclei

    NASA Technical Reports Server (NTRS)

    Hemenway, C. L.

    1973-01-01

    Two sounding rocket payloads were launched from the ESRO range in Sweden during a noctilucent cloud display. Large numbers of submicron particles were collected, most of which appear to be made up of a high density material coated with a low density material. Typical electron micrographs are shown. Particle chemical compositions have been measured by use of dispersive X-ray analysis equipment attached to an electron microscope and have revealed that most of the high density particle nuclei have atomic weights greater than iron.

  18. Bimetallic Platinum-Rhodium Alloy Nanodendrites as Highly Active Electrocatalyst for the Ethanol Oxidation Reaction.

    PubMed

    Bai, Juan; Xiao, Xue; Xue, Yuan-Yuan; Jiang, Jia-Xing; Zeng, Jing-Hui; Li, Xi-Fei; Chen, Yu

    2018-06-13

    Rationally designing and manipulating composition and morphology of precious metal-based bimetallic nanostructures can markedly enhance their electrocatalytic performance, including selectivity, activity, and durability. We herein report the synthesis of bimetallic PtRh alloy nanodendrites (ANDs) with tunable composition by a facile complex-reduction synthetic method under hydrothermal conditions. The structural/morphologic features, formation mechanism, and electrocatalytic performance of PtRh ANDs are investigated thoroughly by various physical characterization and electrochemical methods. The preformed Rh crystal nuclei effectively catalyze the reduction of Pt 2+ precursor, resulting in PtRh alloy generation due to the catalytic growth and atoms interdiffusion process. The Pt atoms deposition distinctly interferes in Rh atoms deposition on Rh crystal nuclei, resulting in dendritic morphology of PtRh ANDs. For the ethanol oxidation reaction (EOR), PtRh ANDs display the chemical composition and solution pH co-dependent electrocatalytic activity. Because of the alloy effect and particular morphologic feature, Pt 1 Rh 1 ANDs with optimized composition exhibit better reactivity and stability for the EOR than commercial Pt nanocrystals electrocatalyst.

  19. Isobar analog states (IAS), double isobar analog states (DIAS), configuration states (CS), and double configuration states (DCS) in halo nuclei. Halo isomers

    NASA Astrophysics Data System (ADS)

    Izosimov, I. N.

    2015-10-01

    It has been shown that IAS, DIAS, CS, and DCS can simultaneously have n-n, n-p, and p-p halo components in their wave functions. Differences in halo structure of the excited and ground states can result in the formation of isomers (halo-isomers). Both the Borromean and tango halo types can be observed for n-p configurations of atomic nuclei. The structure of the ground and excited states with different isospin quantum number in halo like nuclei is discussed. B(Mλ) and B(Eλ) for γ-transitions in 6,7,8Li, 8,9,10Be, 8,10,11B, 10,11,12,13,14C, 13,14,15,16,17N, 15,16,17,19O, and 17F are analyzed. Special attention is given to nuclei whose ground state does not exhibit halo structure but the excited state may have one.

  20. The volatile composition of comets

    NASA Technical Reports Server (NTRS)

    Weaver, H. A.

    1988-01-01

    Comets may be our best probes of the physical and chemical conditions in the outer regions of the solar nebula during that crucial period when the planets formed. The volatile composition of cometary nuclei can be used to decide whether comets are the product of a condensation sequence similar to that invoked to explain the compositions of the planets and asteroids, or if comets are simply agglomerations of interstellar grains which have been insignificantly modified by the events that shaped the other bodies in the solar system. Although cometary nuclei are not generally accessible to observation, observations of cometary comae can illuminate at least some of the mysteries of the nuclei provided one has a detailed knowledge of the excitation conditions in the coma and also has access to basic atomic and molecular data on the many species present in comets. Examined here is the status of our knowledge of the volatile composition of cometary nuclei and how these data are obtained.

  1. THE RADIATIVE NEUTRON CAPTURE ON 2H, 6Li, 7Li, 12C AND 13C AT ASTROPHYSICAL ENERGIES

    NASA Astrophysics Data System (ADS)

    Dubovichenko, Sergey; Dzhazairov-Kakhramanov, Albert; Burkova, Natalia

    2013-05-01

    The continued interest in the study of radiative neutron capture on atomic nuclei is due, on the one hand, to the important role played by this process in the analysis of many fundamental properties of nuclei and nuclear reactions, and, on the other hand, to the wide use of the capture cross-section data in the various applications of nuclear physics and nuclear astrophysics, and, also, to the importance of the analysis of primordial nucleosynthesis in the Universe. This paper is devoted to the description of results for the processes of the radiative neutron capture on certain light atomic nuclei at thermal and astrophysical energies. The consideration of these processes is done within the framework of the potential cluster model (PCM), general description of which was given earlier. The methods of usage of the results obtained, based on the phase shift analysis intercluster potentials, are demonstrated in calculations of the radiative capture characteristics. The considered capture reactions are not part of stellar thermonuclear cycles, but involve in the basic reaction chain of primordial nucleosynthesis in the course of the Universe formation.

  2. Noise suppression for the differential detection in nuclear magnetic resonance gyroscope

    NASA Astrophysics Data System (ADS)

    Yang, Dan; Zhou, Binquan; Chen, LinLin; Jia, YuChen; Lu, QiLin

    2017-10-01

    The nuclear magnetic resonance gyroscope is based on spin-exchange optical pumping of noble gases to detect and measure the angular velocity of the carrier, but it would be challenging to measure the precession signal of noble gas nuclei directly. To solve the problem, the primary detection method utilizes alkali atoms, the precession of nuclear magnetization modulates the alkali atoms at the Larmor frequency of nuclei, relatively speaking, and it is easier to detect the precession signal of alkali atoms. The precession frequency of alkali atoms is detected by the rotation angle of linearly polarized probe light; and differential detection method is commonly used in NMRG in order to detect the linearly polarized light rotation angle. Thus, the detection accuracy of differential detection system will affect the sensitivity of the NMRG. For the purpose of further improvement of the sensitivity level of the NMRG, this paper focuses on the aspects of signal detection, and aims to do an error analysis as well as an experimental research of the linearly light rotation angle detection. Through the theoretical analysis and the experimental illustration, we found that the extinction ratio σ2 and DC bias are the factors that will produce detective noise in the differential detection method.

  3. Shell Corrections Stabilizing Superheavy Nuclei and Semi-spheroidal Atomic Clusters

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Poenaru, Dorin N.

    2008-01-24

    The macroscopic-microscopic method is used to illustrate the shell effect stabilizing superheavy nuclei and to study the stability of semi-spheroidal clusters deposited on planar surfaces. The alpha decay of superheavy nuclei is calculated using three models: the analytical superasymmetric fission model; the universal curve, and the semiempirical formula taking into account the shell effects. Analytical relationships are obtained for the energy levels of the new semi-spheroidal harmonic oscillator (SSHO) single-particle model and for the surface and curvature energies of the semi-spheroidal clusters. The maximum degeneracy of the SSHO is reached at a super-deformed prolate shape for which the minimum ofmore » the liquid drop model energy is also attained.« less

  4. The energy distribution of very heavy cosmic ray nuclei within the penumbra at Palestine, Texas

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Mathiesen, O.; Larsson, L.; Andersson, R.

    1975-09-01

    The low-energy end of the rigidity spectrum of cosmic ray nuclei with atomic numbers 7greater than or equal to18, recorded in a balloon flight conducted from Palestine, Texas, has been compared with a corresponding theoretical spectrum based on the computations by Shea and Smart. The two distributions are found to be in qualitative agreement with each other. The spread in apparent particle charge, caused by the theoretical distribution of particle velocity at Palestine, has been calculated for detectors with different response functions. The resulting structure of the predicted charge spectrum of iron group nuclei is found to be in goodmore » agreement with corresponding experimental data.« less

  5. Facile synthesis of graphene on dielectric surfaces using a two-temperature reactor CVD system

    NASA Astrophysics Data System (ADS)

    Zhang, C.; Man, B. Y.; Yang, C.; Jiang, S. Z.; Liu, M.; Chen, C. S.; Xu, S. C.; Sun, Z. C.; Gao, X. G.; Chen, X. J.

    2013-10-01

    Direct deposition of graphene on a dielectric substrate is demonstrated using a chemical vapor deposition system with a two-temperature reactor. The two-temperature reactor is utilized to offer sufficient, well-proportioned floating Cu atoms and to provide a temperature gradient for facile synthesis of graphene on dielectric surfaces. The evaporated Cu atoms catalyze the reaction in the presented method. C atoms and Cu atoms respectively act as the nuclei for forming graphene film in the low-temperature zone and the zones close to the high-temperature zones. A uniform and high-quality graphene film is formed in an atmosphere of sufficient and well-proportioned floating Cu atoms. Raman spectroscopy, scanning electron microscopy and atomic force microscopy confirm the presence of uniform and high-quality graphene.

  6. Electric Dipole Moment Measurements with Rare Isotopes

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Chupp, Timothy

    The origin of matter is one of the deepest questions addressed by science and remains a mystery because our understanding of the Big Bang suggests that equal amounts of matter as antimatter would be created and annihilate leaving nothing from which stars, galaxies, planets and ultimately life as we know it was created. We know this is not the case in the universe, and so the explanation that the laws of physics can distinguish the difference of moving forward and backward in time and provide mechanisms that produce more matter that antimatter so that a little bit was left over.more » These same laws of physics affect our world today and would very slightly change the shape of an atom, stretching is along the direction of the spin of its nucleus. This subtle shape change has been searched in many systems - the neutron, atoms and molecules, but has not yet been detected, even as the motivation is strengthened by our understanding of their structure. We therefore look to new systems that have special features that make these effects stand out. Rare isotopes provide one possibility and specific radon atoms are our choice. We have developed techniques to make these measurements with short-lived radioactive atoms, studied the nuclei to provide deeper understanding of how these affect arise in such atoms (including radium) and developed new laser-based techniques to measure and control the magnetic fields necessary to perform these exquisitely sensitive measurements. In this work we have shown that radioactive radon atoms can be produced and transported to an apparatus that lines up the spins of the atoms. We have also shown that the nuclei of nearby radium are pear shaped and that the radon nuclei likely oscillate from one pear shape to its mirror reflection. We have also used the techniques which control nuclear spin to study the magnetic environment in a magnetically shielded room, which has the smallest magnetic field in a large volume in the universe. Measuring magnetic fields and detecting noble atoms' shapes using lasers will provide new techniques for these measurements and impact a broad range of applications including measurements of the neutron EDM. Harvesting rare isotopes at the future FRIB facility at Michigan State University will provide much stronger sources of the isotopes of radon and radium for future-generation experiments and also provide new isotopes for applications including medicine.« less

  7. The Development of Materials for Structures and Radiation Shielding in Aerospace

    NASA Technical Reports Server (NTRS)

    Kiefer, Richard L.; Orwoll, Robert A.

    2001-01-01

    Polymeric materials on space vehicles and high-altitude aircraft win be exposed to highly penetrating radiations. These radiations come from solar flares and galactic cosmic rays (GCR). Radiation from solar flares consists primarily of protons with energies less than 1 GeV. On the other hand, GCR consist of nuclei with energies as high as 10(exp 10) GeV. Over 90% of the nuclei in GCR are protons and alpha particles, however there is a small but significant component of particles with atomic numbers greater than ten. Particles with high atomic number (Z) and high energy interact with very high specific ionization and thus represent a serious hazard for humans and electronic equipment on a spacecraft or on high-altitude commercial aircraft (most importantly for crew members who would have long exposures). Neutrons generated by reactions with the high energy particles also represent a hazard both for humans and electronic equipment.

  8. Comparison of experimental and theoretical electron-impact-ionization triple-differential cross sections for ethane

    NASA Astrophysics Data System (ADS)

    Ali, Esam; Nixon, Kate; Murray, Andrew; Ning, Chuangang; Colgan, James; Madison, Don

    2015-10-01

    We have recently examined electron-impact ionization of molecules that have one large atom at the center, surrounded by H nuclei (H2O , N H3 , C H4 ). All of these molecules have ten electrons; however, they vary in their molecular symmetry. We found that the triple-differential cross sections (TDCSs) for the highest occupied molecular orbitals (HOMOs) were similar, as was the character of the HOMO orbitals which had a p -type "peanut" shape. In this work, we examine ethane (C2H6 ) which is a molecule that has two large atoms surrounded by H nuclei, so that its HOMO has a double-peanut shape. The experiment was performed using a coplanar symmetric geometry (equal final-state energies and angles). We find the TDCS for ethane is similar to the single-center molecules at higher energies, and is similar to a diatomic molecule at lower energies.

  9. The Superheavy Elements and Anti-Gravity

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Anastasovski, Petar K.

    2004-02-04

    The essence of any propulsion concept is to overcome gravity. Anti-gravity is a natural means to achieve this. Thus, the technology to pursue anti-gravity, by using superheavy elements, may provide a new propulsion paradigm. The theory of superluminal relativity provides a hypothesis for existence of elements with atomic number up to Z = 145, some of which may possess anti-gravity properties. Analysis results show that curved space-time exists demonstrating both gravitic and anti-gravitic properties not only around nuclei but inside the nuclei as well. Two groups of elements (Z < 64 and 63 < Z <145) exist that demonstrate thesemore » capabilities. The nuclei of the first group of elements have the masses with only the property of gravity. The nuclei of the elements of the second group have the masses with both properties: gravity and anti-gravity in two different ranges of curved space-time around the nuclei.. The hypothetical element with Z = 145 is the unique among all elements whose nucleus has only anti-gravity property. It is proposed that this element be named Hawking, in honour of Stephen W. Hawking.« less

  10. The Superheavy Elements and Anti-Gravity

    NASA Astrophysics Data System (ADS)

    Anastasovski, Petar K.

    2004-02-01

    The essence of any propulsion concept is to overcome gravity. Anti-gravity is a natural means to achieve this. Thus, the technology to pursue anti-gravity, by using superheavy elements, may provide a new propulsion paradigm. The theory of superluminal relativity provides a hypothesis for existence of elements with atomic number up to Z = 145, some of which may possess anti-gravity properties. Analysis results show that curved space-time exists demonstrating both gravitic and anti-gravitic properties not only around nuclei but inside the nuclei as well. Two groups of elements (Z < 64 and 63 < Z <145) exist that demonstrate these capabilities. The nuclei of the first group of elements have the masses with only the property of gravity. The nuclei of the elements of the second group have the masses with both properties: gravity and anti-gravity in two different ranges of curved space-time around the nuclei.. The hypothetical element with Z = 145 is the unique among all elements whose nucleus has only anti-gravity property. It is proposed that this element be named Hawking, in honour of Stephen W. Hawking.

  11. Structural studies of chromatin and chromosomes. Progress report, March 15--September 15, 1997

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Bradbury, E.M.

    This study focused on the following: (1) the structure of chromatin and chromosomes by neutron and x-ray scatter and atomic force microscope; (2) the architecture of human sperm and the structure of sperm by atomic force microscopy (AFM); (3) genome-architecture and higher-order structures in human sperm nuclei; and (4) the effects of histone modifications on the structure of nucleosomes by protein DNA crosslinking method.

  12. Incorporating nuclear vibrational energies into the "atom in molecules" analysis: An analytical study

    NASA Astrophysics Data System (ADS)

    Gharabaghi, Masumeh; Shahbazian, Shant

    2017-04-01

    The quantum theory of atoms in molecules (QTAIM) is based on the clamped nucleus paradigm and solely working with the electronic wavefunctions, so does not include nuclear vibrations in the AIM analysis. On the other hand, the recently extended version of the QTAIM, called the multi-component QTAIM (MC-QTAIM), incorporates both electrons and quantum nuclei, i.e., those nuclei treated as quantum waves instead of clamped point charges, into the AIM analysis using non-adiabatic wavefunctions. Thus, the MC-QTAIM is the natural framework to incorporate the role of nuclear vibrations into the AIM analysis. In this study, within the context of the MC-QTAIM, the formalism of including nuclear vibrational energy in the atomic basin energy is developed in detail and its contribution is derived analytically using the recently proposed non-adiabatic Hartree product nuclear wavefunction. It is demonstrated that within the context of this wavefunction, the quantum nuclei may be conceived pseudo-adiabatically as quantum oscillators and both isotropic harmonic and anisotropic anharmonic oscillator models are used to compute the zero-point nuclear vibrational energy contribution to the basin energies explicitly. Inspired by the results gained within the context of the MC-QTAIM analysis, a heuristic approach is proposed within the context of the QTAIM to include nuclear vibrational energy in the basin energy from the vibrational wavefunction derived adiabatically. The explicit calculation of the basin contribution of the zero-point vibrational energy using the uncoupled harmonic oscillator model leads to results consistent with those derived from the MC-QTAIM.

  13. Incorporating nuclear vibrational energies into the "atom in molecules" analysis: An analytical study.

    PubMed

    Gharabaghi, Masumeh; Shahbazian, Shant

    2017-04-21

    The quantum theory of atoms in molecules (QTAIM) is based on the clamped nucleus paradigm and solely working with the electronic wavefunctions, so does not include nuclear vibrations in the AIM analysis. On the other hand, the recently extended version of the QTAIM, called the multi-component QTAIM (MC-QTAIM), incorporates both electrons and quantum nuclei, i.e., those nuclei treated as quantum waves instead of clamped point charges, into the AIM analysis using non-adiabatic wavefunctions. Thus, the MC-QTAIM is the natural framework to incorporate the role of nuclear vibrations into the AIM analysis. In this study, within the context of the MC-QTAIM, the formalism of including nuclear vibrational energy in the atomic basin energy is developed in detail and its contribution is derived analytically using the recently proposed non-adiabatic Hartree product nuclear wavefunction. It is demonstrated that within the context of this wavefunction, the quantum nuclei may be conceived pseudo-adiabatically as quantum oscillators and both isotropic harmonic and anisotropic anharmonic oscillator models are used to compute the zero-point nuclear vibrational energy contribution to the basin energies explicitly. Inspired by the results gained within the context of the MC-QTAIM analysis, a heuristic approach is proposed within the context of the QTAIM to include nuclear vibrational energy in the basin energy from the vibrational wavefunction derived adiabatically. The explicit calculation of the basin contribution of the zero-point vibrational energy using the uncoupled harmonic oscillator model leads to results consistent with those derived from the MC-QTAIM.

  14. L. James Rainwater and the Atomic Nuclei

    Science.gov Websites

    described the experimental situation for nuclear quadrupole moments. It was a fortuitous situation made even given value after a lapse of time. Top Some links on this page may take you to non-federal websites

  15. Relativistic well-tempered Gaussian basis sets for helium through mercury

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Okada, S.; Matsuoka, O.

    1989-10-01

    Exponent parameters of the nonrelativistically optimized well-tempered Gaussian basis sets of Huzinaga and Klobukowski have been employed for Dirac--Fock--Roothaan calculations without their reoptimization. For light atoms He (atomic number {ital Z}=2)--Rh ({ital Z}=45), the number of exponent parameters used has been the same as the nonrelativistic basis sets and for heavier atoms Pd ({ital Z}=46)--Hg({ital Z}=80), two 2{ital p} (and three 3{ital d}) Gaussian basis functions have been augmented. The scheme of kinetic energy balance and the uniformly charged sphere model of atomic nuclei have been adopted. The qualities of the calculated basis sets are close to the Dirac--Fock limit.

  16. Measurement of elliptic flow of light nuclei at √{sN N}=200 , 62.4, 39, 27, 19.6, 11.5, and 7.7 GeV at the BNL Relativistic Heavy Ion Collider

    NASA Astrophysics Data System (ADS)

    Adamczyk, L.; Adkins, J. K.; Agakishiev, G.; Aggarwal, M. M.; Ahammed, Z.; Alekseev, I.; Aparin, A.; Arkhipkin, D.; Aschenauer, E. C.; Attri, A.; Averichev, G. S.; Bai, X.; Bairathi, V.; Bellwied, R.; Bhasin, A.; Bhati, A. K.; Bhattarai, P.; Bielcik, J.; Bielcikova, J.; Bland, L. C.; Bordyuzhin, I. G.; Bouchet, J.; Brandenburg, J. D.; Brandin, A. V.; Bunzarov, I.; Butterworth, J.; Caines, H.; Calderón de la Barca Sánchez, M.; Campbell, J. M.; Cebra, D.; Chakaberia, I.; Chaloupka, P.; Chang, Z.; Chatterjee, A.; Chattopadhyay, S.; Chen, J. H.; Chen, X.; Cheng, J.; Cherney, M.; Christie, W.; Contin, G.; Crawford, H. J.; Das, S.; De Silva, L. C.; Debbe, R. R.; Dedovich, T. G.; Deng, J.; Derevschikov, A. A.; di Ruzza, B.; Didenko, L.; Dilks, C.; Dong, X.; Drachenberg, J. L.; Draper, J. E.; Du, C. M.; Dunkelberger, L. E.; Dunlop, J. C.; Efimov, L. G.; Engelage, J.; Eppley, G.; Esha, R.; Evdokimov, O.; Eyser, O.; Fatemi, R.; Fazio, S.; Federic, P.; Fedorisin, J.; Feng, Z.; Filip, P.; Fisyak, Y.; Flores, C. E.; Fulek, L.; Gagliardi, C. A.; Garand, D.; Geurts, F.; Gibson, A.; Girard, M.; Greiner, L.; Grosnick, D.; Gunarathne, D. S.; Guo, Y.; Gupta, S.; Gupta, A.; Guryn, W.; Hamad, A. I.; Hamed, A.; Haque, R.; Harris, J. W.; He, L.; Heppelmann, S.; Heppelmann, S.; Hirsch, A.; Hoffmann, G. W.; Horvat, S.; Huang, T.; Huang, X.; Huang, B.; Huang, H. Z.; Huck, P.; Humanic, T. J.; Igo, G.; Jacobs, W. W.; Jang, H.; Jentsch, A.; Jia, J.; Jiang, K.; Judd, E. G.; Kabana, S.; Kalinkin, D.; Kang, K.; Kauder, K.; Ke, H. W.; Keane, D.; Kechechyan, A.; Khan, Z. H.; Kikoła, D. P.; Kisel, I.; Kisiel, A.; Kochenda, L.; Koetke, D. D.; Kosarzewski, L. K.; Kraishan, A. F.; Kravtsov, P.; Krueger, K.; Kumar, L.; Lamont, M. A. C.; Landgraf, J. M.; Landry, K. D.; Lauret, J.; Lebedev, A.; Lednicky, R.; Lee, J. H.; Li, X.; Li, C.; Li, X.; Li, Y.; Li, W.; Lin, T.; Lisa, M. A.; Liu, F.; Ljubicic, T.; Llope, W. J.; Lomnitz, M.; Longacre, R. S.; Luo, X.; Ma, R.; Ma, G. L.; Ma, Y. G.; Ma, L.; Magdy, N.; Majka, R.; Manion, A.; Margetis, S.; Markert, C.; Matis, H. S.; McDonald, D.; McKinzie, S.; Meehan, K.; Mei, J. C.; Minaev, N. G.; Mioduszewski, S.; Mishra, D.; Mohanty, B.; Mondal, M. M.; Morozov, D. A.; Mustafa, M. K.; Nandi, B. K.; Nasim, Md.; Nayak, T. K.; Nigmatkulov, G.; Niida, T.; Nogach, L. V.; Noh, S. Y.; Novak, J.; Nurushev, S. B.; Odyniec, G.; Ogawa, A.; Oh, K.; Okorokov, V. A.; Olvitt, D.; Page, B. S.; Pak, R.; Pan, Y. X.; Pandit, Y.; Panebratsev, Y.; Pawlik, B.; Pei, H.; Perkins, C.; Pile, P.; Pluta, J.; Poniatowska, K.; Porter, J.; Posik, M.; Poskanzer, A. M.; Pruthi, N. K.; Putschke, J.; Qiu, H.; Quintero, A.; Ramachandran, S.; Raniwala, R.; Raniwala, S.; Ray, R. L.; Ritter, H. G.; Roberts, J. B.; Rogachevskiy, O. V.; Romero, J. L.; Ruan, L.; Rusnak, J.; Rusnakova, O.; Sahoo, N. R.; Sahu, P. K.; Sakrejda, I.; Salur, S.; Sandweiss, J.; Sarkar, A.; Schambach, J.; Scharenberg, R. P.; Schmah, A. M.; Schmidke, W. B.; Schmitz, N.; Seger, J.; Seyboth, P.; Shah, N.; Shahaliev, E.; Shanmuganathan, P. V.; Shao, M.; Sharma, M. K.; Sharma, B.; Shen, W. Q.; Shi, Z.; Shi, S. S.; Shou, Q. Y.; Sichtermann, E. P.; Sikora, R.; Simko, M.; Singha, S.; Skoby, M. J.; Smirnov, N.; Smirnov, D.; Solyst, W.; Song, L.; Sorensen, P.; Spinka, H. M.; Srivastava, B.; Stanislaus, T. D. S.; Stepanov, M.; Stock, R.; Strikhanov, M.; Stringfellow, B.; Sumbera, M.; Summa, B.; Sun, X. M.; Sun, Z.; Sun, Y.; Surrow, B.; Svirida, D. N.; Tang, Z.; Tang, A. H.; Tarnowsky, T.; Tawfik, A.; Thäder, J.; Thomas, J. H.; Timmins, A. R.; Tlusty, D.; Todoroki, T.; Tokarev, M.; Trentalange, S.; Tribble, R. E.; Tribedy, P.; Tripathy, S. K.; Tsai, O. D.; Ullrich, T.; Underwood, D. G.; Upsal, I.; Van Buren, G.; van Nieuwenhuizen, G.; Vandenbroucke, M.; Varma, R.; Vasiliev, A. N.; Vertesi, R.; Videbæk, F.; Vokal, S.; Voloshin, S. A.; Vossen, A.; Wang, Y.; Wang, G.; Wang, J. S.; Wang, H.; Wang, Y.; Wang, F.; Webb, G.; Webb, J. C.; Wen, L.; Westfall, G. D.; Wieman, H.; Wissink, S. W.; Witt, R.; Wu, Y.; Xiao, Z. G.; Xie, W.; Xie, G.; Xin, K.; Xu, H.; Xu, Z.; Xu, J.; Xu, Y. F.; Xu, Q. H.; Xu, N.; Yang, Y.; Yang, S.; Yang, C.; Yang, Y.; Yang, Y.; Yang, Q.; Ye, Z.; Ye, Z.; Yepes, P.; Yi, L.; Yip, K.; Yoo, I.-K.; Yu, N.; Zbroszczyk, H.; Zha, W.; Zhang, J.; Zhang, Y.; Zhang, X. P.; Zhang, Z.; Zhang, J. B.; Zhang, S.; Zhang, S.; Zhang, J.; Zhao, J.; Zhong, C.; Zhou, L.; Zhu, X.; Zoulkarneeva, Y.; Zyzak, M.; STAR Collaboration

    2016-09-01

    We present measurements of second-order azimuthal anisotropy (v2) at midrapidity (|y |<1.0 ) for light nuclei d ,t ,3He (for √{sN N}=200 , 62.4, 39, 27, 19.6, 11.5, and 7.7 GeV) and antinuclei d ¯ (√{sN N}=200 , 62.4, 39, 27, and 19.6 GeV) and ¯3He (√{sN N}=200 GeV) in the STAR (Solenoidal Tracker at RHIC) experiment. The v2 for these light nuclei produced in heavy-ion collisions is compared with those for p and p ¯. We observe mass ordering in nuclei v2(pT) at low transverse momenta (pT<2.0 GeV/c ). We also find a centrality dependence of v2 for d and d ¯. The magnitude of v2 for t and 3He agree within statistical errors. Light-nuclei v2 are compared with predictions from a blast-wave model. Atomic mass number (A ) scaling of light-nuclei v2(pT) seems to hold for pT/A <1.5 GeV /c . Results on light-nuclei v2 from a transport-plus-coalescence model are consistent with the experimental measurements.

  17. Measurement of elliptic flow of light nuclei at s N N = 200 , 62.4, 39, 27, 19.6, 11.5, and 7.7 GeV at the BNL Relativistic Heavy Ion Collider

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Adamczyk, L.; Adkins, J. K.; Agakishiev, G.

    Here we present measurements of second-order azimuthal anisotropy ( v 2 ) at midrapidity ( |y| < 1.0 ) for light nuclei d , t , 3He (formore » $$\\sqrt{s}$$$_{NN}$$ = 200 , 62.4, 39, 27, 19.6, 11.5, and 7.7 GeV) and antinuclei$$\\bar{d}$$ ( $$\\sqrt{s}$$$_{NN}$$ = 200 , 62.4, 39, 27, and 19.6 GeV) and 3 ¯¯¯¯¯ He ( $$\\sqrt{s}$$$_{NN}$$ = 200 GeV) in the STAR (Solenoidal Tracker at RHIC) experiment. The v 2 for these light nuclei produced in heavy-ion collisions is compared with those for p and $$\\bar{p}$$. We observe mass ordering in nuclei v 2 ( p T) at low transverse momenta ( p T < 2.0 GeV/c). We also find a centrality dependence of v 2 for d and $$\\bar{d}$$ . The magnitude of v 2 for t and 3He agree within statistical errors. Light-nuclei v 2 are compared with predictions from a blast-wave model. Atomic mass number ( A ) scaling of light-nuclei v 2 (p T) seems to hold for p T / A < 1.5 GeV/c . Results on light-nuclei v 2 from a transport-plus-coalescence model are consistent with the experimental measurements.« less

  18. Measurement of elliptic flow of light nuclei at s N N = 200 , 62.4, 39, 27, 19.6, 11.5, and 7.7 GeV at the BNL Relativistic Heavy Ion Collider

    DOE PAGES

    Adamczyk, L.; Adkins, J. K.; Agakishiev, G.; ...

    2016-09-23

    Here we present measurements of second-order azimuthal anisotropy ( v 2 ) at midrapidity ( |y| < 1.0 ) for light nuclei d , t , 3He (formore » $$\\sqrt{s}$$$_{NN}$$ = 200 , 62.4, 39, 27, 19.6, 11.5, and 7.7 GeV) and antinuclei$$\\bar{d}$$ ( $$\\sqrt{s}$$$_{NN}$$ = 200 , 62.4, 39, 27, and 19.6 GeV) and 3 ¯¯¯¯¯ He ( $$\\sqrt{s}$$$_{NN}$$ = 200 GeV) in the STAR (Solenoidal Tracker at RHIC) experiment. The v 2 for these light nuclei produced in heavy-ion collisions is compared with those for p and $$\\bar{p}$$. We observe mass ordering in nuclei v 2 ( p T) at low transverse momenta ( p T < 2.0 GeV/c). We also find a centrality dependence of v 2 for d and $$\\bar{d}$$ . The magnitude of v 2 for t and 3He agree within statistical errors. Light-nuclei v 2 are compared with predictions from a blast-wave model. Atomic mass number ( A ) scaling of light-nuclei v 2 (p T) seems to hold for p T / A < 1.5 GeV/c . Results on light-nuclei v 2 from a transport-plus-coalescence model are consistent with the experimental measurements.« less

  19. The Ehrenfest force field: Topology and consequences for the definition of an atom in a molecule.

    PubMed

    Martín Pendás, A; Hernández-Trujillo, J

    2012-10-07

    The Ehrenfest force is the force acting on the electrons in a molecule due to the presence of the other electrons and the nuclei. There is an associated force field in three-dimensional space that is obtained by the integration of the corresponding Hermitian quantum force operator over the spin coordinates of all of the electrons and the space coordinates of all of the electrons but one. This paper analyzes the topology induced by this vector field and its consequences for the definition of molecular structure and of an atom in a molecule. Its phase portrait reveals: that the nuclei are attractors of the Ehrenfest force, the existence of separatrices yielding a dense partitioning of three-dimensional space into disjoint regions, and field lines connecting the attractors through these separatrices. From the numerical point of view, when the Ehrenfest force field is obtained as minus the divergence of the kinetic stress tensor, the induced topology was found to be highly sensitive to choice of gaussian basis sets at long range. Even the use of large split valence and highly uncontracted basis sets can yield spurious critical points that may alter the number of attraction basins. Nevertheless, at short distances from the nuclei, in general, the partitioning of three-dimensional space with the Ehrenfest force field coincides with that induced by the gradient field of the electron density. However, exceptions are found in molecules where the electron density yields results in conflict with chemical intuition. In these cases, the molecular graphs of the Ehrenfest force field reveal the expected atomic connectivities. This discrepancy between the definition of an atom in a molecule between the two vector fields casts some doubts on the physical meaning of the integration of Ehrenfest forces over the basins of the electron density.

  20. On the existence of Rydberg nuclear molecules

    NASA Astrophysics Data System (ADS)

    Bertulani, C. A.; Frederico, T.; Hussein, M. S.

    2017-11-01

    Present nuclear detection techniques prevents us from determining if the analogue of a Rydberg molecule exists for the nuclear case. But nothing in nature disallows their existence. As in the atomic case, Rydberg nuclear molecules would be a laboratory for new aspects and applications of nuclear physics. We propose that Rydberg nuclear molecules, which represent the exotic, halo nuclei version, such as 11Be +11Be, of the well known quasimolecules observed in stable nuclei such as 12C +12C, might be common structures that could manifest their existence along the dripline. A study of possible candidates and the expected structure of such exotic clustering of two halo nuclei: the Rydberg nuclear molecules, is made on the basis of three different methods. It is shown that such cluster structures might be stable and unexpectedly common.

  1. Rules governing the composition of revolving clusters in quasiband and prolate-deformation states of atomic nuclei

    PubMed Central

    Pauling, Linus

    1982-01-01

    A set of rules, involving the magic and semimagic values of neutron and proton numbers and the proton/neutron ratio, is formulated for the composition of the revolving clusters producing the values of the moment of inertia given by the differences in energy of the adjacent levels in quasibands and bands of nuclei. The cluster compositions assigned with use of these rules to isotopes of Kr, Sr, Zr, Mo, and the actinon nuclei and to successive levels of the ground-state band of 158Er lead to reasonable values of the radius of revolution (the distance from the center of the nonrevolving sphere to the center of the cluster). These values correspond to a spheron diameter of about 3.20 fm. PMID:16593256

  2. Elementary Particles and Forces.

    ERIC Educational Resources Information Center

    Quigg, Chris

    1985-01-01

    Discusses subatomic particles (quarks, leptons, and others) revealed by higher accelerator energies. A connection between forces at this subatomic level has been established, and prospects are good for a description of forces that encompass binding atomic nuclei. Colors, fundamental interactions, screening, camouflage, electroweak symmetry, and…

  3. Method and apparatus for transmutation of atomic nuclei

    DOEpatents

    Maenchen, John Eric; Ruiz, Carlos Leon

    1998-01-01

    Insuring a constant supply of radioisotopes is of great importance to medicine and industry. This invention addresses this problem, and helps to solve it by introducing a new apparatus for transmutation of isotopes which enables swift and flexible production on demand.

  4. Nuclear equation of state from ground and collective excited state properties of nuclei

    NASA Astrophysics Data System (ADS)

    Roca-Maza, X.; Paar, N.

    2018-07-01

    This contribution reviews the present status on the available constraints to the nuclear equation of state (EoS) around saturation density from nuclear structure calculations on ground and collective excited state properties of atomic nuclei. It concentrates on predictions based on self-consistent mean-field calculations, which can be considered as an approximate realization of an exact energy density functional (EDF). EDFs are derived from effective interactions commonly fitted to nuclear masses, charge radii and, in many cases, also to pseudo-data such as nuclear matter properties. Although in a model dependent way, EDFs constitute nowadays a unique tool to reliably and consistently access bulk ground state and collective excited state properties of atomic nuclei along the nuclear chart as well as the EoS. For comparison, some emphasis is also given to the results obtained with the so called ab initio approaches that aim at describing the nuclear EoS based on interactions fitted to few-body data only. Bridging the existent gap between these two frameworks will be essential since it may allow to improve our understanding on the diverse phenomenology observed in nuclei. Examples on observations from astrophysical objects and processes sensitive to the nuclear EoS are also briefly discussed. As the main conclusion, the isospin dependence of the nuclear EoS around saturation density and, to a lesser extent, the nuclear matter incompressibility remain to be accurately determined. Experimental and theoretical efforts in finding and measuring observables specially sensitive to the EoS properties are of paramount importance, not only for low-energy nuclear physics but also for nuclear astrophysics applications.

  5. Effective field theory description of halo nuclei

    NASA Astrophysics Data System (ADS)

    Hammer, H.-W.; Ji, C.; Phillips, D. R.

    2017-10-01

    Nuclear halos emerge as new degrees of freedom near the neutron and proton driplines. They consist of a core and one or a few nucleons which spend most of their time in the classically-forbidden region outside the range of the interaction. Individual nucleons inside the core are thus unresolved in the halo configuration, and the low-energy effective interactions are short-range forces between the core and the valence nucleons. Similar phenomena occur in clusters of 4He atoms, cold atomic gases near a Feshbach resonance, and some exotic hadrons. In these weakly-bound quantum systems universal scaling laws for s-wave binding emerge that are independent of the details of the interaction. Effective field theory (EFT) exposes these correlations and permits the calculation of non-universal corrections to them due to short-distance effects, as well as the extension of these ideas to systems involving the Coulomb interaction and/or binding in higher angular-momentum channels. Halo nuclei exhibit all these features. Halo EFT, the EFT for halo nuclei, has been used to compute the properties of single-neutron, two-neutron, and single-proton halos of s-wave and p-wave type. This review summarizes these results for halo binding energies, radii, Coulomb dissociation, and radiative capture, as well as the connection of these properties to scattering parameters, thereby elucidating the universal correlations between all these observables. We also discuss how Halo EFT's encoding of the long-distance physics of halo nuclei can be used to check and extend ab initio calculations that include detailed modeling of their short-distance dynamics.

  6. Feasibility of Harvesting Radon from FRIB Beam Dump

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Visser, A.; Scielzo, N.

    The observation of a permanent electric dipole moment (EDM) in an atom would signal a long-soughtafter presence of time-reversal violation and would have far reaching consequences for both particle physics and cosmology. Currently, the most stringent limitation on time-reversal violating effects in the nucleus comes from studies of stable 199Hg. However, for certain nuclei which have an octupole deformed shape, such as 223Rn, the time-reversal violating interactions are expected to be 100-1000 times greater than in 199Hg (Auerbach et al. 1996). As a result, there is great interest in searching for EDMs in octupole deformed nuclei and some of themore » initial studies of these nuclei have been featured on the cover of the journal Nature (Gaffney et al. 2013). All the octupole deformed nuclei of interest are radioactive and therefore available only in limited quantities. The primary challenge for an EDM experiment using radon is to collect large enough samples to perform sensitive searches.« less

  7. Isobar analog states (IAS), double isobar analog states (DIAS), configuration states (CS), and double configuration states (DCS) in halo nuclei. Halo isomers

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Izosimov, I. N., E-mail: izosimov@jinr.ru

    2015-10-15

    It has been shown that IAS, DIAS, CS, and DCS can simultaneously have n-n, n-p, and p-p halo components in their wave functions. Differences in halo structure of the excited and ground states can result in the formation of isomers (halo-isomers). Both the Borromean and tango halo types can be observed for n-p configurations of atomic nuclei. The structure of the ground and excited states with different isospin quantum number in halo like nuclei is discussed. B(Mλ) and B(Eλ) for γ-transitions in {sup 6,7,8}Li, {sup 8,9,10}Be, {sup 8,10,11}B, {sup 10,11,12,13,14}C, {sup 13,14,15,16,17}N, {sup 15,16,17,19}O, and {sup 17}F are analyzed. Specialmore » attention is given to nuclei whose ground state does not exhibit halo structure but the excited state may have one.« less

  8. A Molecular–Structure Hypothesis

    PubMed Central

    Boeyens, Jan C. A.

    2010-01-01

    The self-similar symmetry that occurs between atomic nuclei, biological growth structures, the solar system, globular clusters and spiral galaxies suggests that a similar pattern should characterize atomic and molecular structures. This possibility is explored in terms of the current molecular structure-hypothesis and its extension into four-dimensional space-time. It is concluded that a quantum molecule only has structure in four dimensions and that classical (Newtonian) structure, which occurs in three dimensions, cannot be simulated by quantum-chemical computation. PMID:21151437

  9. Quantum molecular dynamics simulations of dense matter

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Collins, L.; Kress, J.; Troullier, N.

    1997-12-31

    The authors have developed a quantum molecular dynamics (QMD) simulation method for investigating the properties of dense matter in a variety of environments. The technique treats a periodically-replicated reference cell containing N atoms in which the nuclei move according to the classical equations-of-motion. The interatomic forces are generated from the quantum mechanical interactions of the (between?) electrons and nuclei. To generate these forces, the authors employ several methods of varying sophistication from the tight-binding (TB) to elaborate density functional (DF) schemes. In the latter case, lengthy simulations on the order of 200 atoms are routinely performed, while for the TB,more » which requires no self-consistency, upwards to 1000 atoms are systematically treated. The QMD method has been applied to a variety cases: (1) fluid/plasma Hydrogen from liquid density to 20 times volume-compressed for temperatures of a thousand to a million degrees Kelvin; (2) isotopic hydrogenic mixtures, (3) liquid metals (Li, Na, K); (4) impurities such as Argon in dense hydrogen plasmas; and (5) metal/insulator transitions in rare gas systems (Ar,Kr) under high compressions. The advent of parallel versions of the methods, especially for fast eigensolvers, presage LDA simulations in the range of 500--1000 atoms and TB runs for tens of thousands of particles. This leap should allow treatment of shock chemistry as well as large-scale mixtures of species in highly transient environments.« less

  10. Benchmark calculations of excess electrons in water cluster cavities: balancing the addition of atom-centered diffuse functions versus floating diffuse functions.

    PubMed

    Zhang, Changzhe; Bu, Yuxiang

    2016-09-14

    Diffuse functions have been proved to be especially crucial for the accurate characterization of excess electrons which are usually bound weakly in intermolecular zones far away from the nuclei. To examine the effects of diffuse functions on the nature of the cavity-shaped excess electrons in water cluster surroundings, both the HOMO and LUMO distributions, vertical detachment energies (VDEs) and visible absorption spectra of two selected (H2O)24(-) isomers are investigated in the present work. Two main types of diffuse functions are considered in calculations including the Pople-style atom-centered diffuse functions and the ghost-atom-based floating diffuse functions. It is found that augmentation of atom-centered diffuse functions contributes to a better description of the HOMO (corresponding to the VDE convergence), in agreement with previous studies, but also leads to unreasonable diffuse characters of the LUMO with significant red-shifts in the visible spectra, which is against the conventional point of view that the more the diffuse functions, the better the results. The issue of designing extra floating functions for excess electrons has also been systematically discussed, which indicates that the floating diffuse functions are necessary not only for reducing the computational cost but also for improving both the HOMO and LUMO accuracy. Thus, the basis sets with a combination of partial atom-centered diffuse functions and floating diffuse functions are recommended for a reliable description of the weakly bound electrons. This work presents an efficient way for characterizing the electronic properties of weakly bound electrons accurately by balancing the addition of atom-centered diffuse functions and floating diffuse functions and also by balancing the computational cost and accuracy of the calculated results, and thus is very useful in the relevant calculations of various solvated electron systems and weakly bound anionic systems.

  11. Atomic spectrometry update - atomic mass spectrometry.

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Bacon, J.; Crain, J. S.; McMahon, A. W.

    The MS and XRF updates have been published together since their introduction in 1988. In the last few years, however, the two sections have been prepared independently of each other and it therefore seemed appropriate to publish the two sections separately. With effect from this issue, the MS Update will appear in the October issue of JAAS and the XRF Update in the November issue. The format used for the MS section is broadly similar to that used last year, with some additional sub-headings. This Update is intended to cover all atomic and stable isotopic MS techniques, but not thosemore » used in studies of fundamental nuclear physics and exotic nuclei far from stability. Also excluded are those reports in which MS is used as a tool in the study of molecular processes and of gaseous components. the review is based on critical selection of developments in instrumentation and methodology, notable for their innovation, originality or achievement of significant advances, and is not intended to be comprehensive in its coverage. Conference papers are only included if they contain enough information to show they meet these criteria, and our policy in general remains one of waiting for a development to appear in a full paper before inclusion in the review. a similar policy applies to foreign language papers unlikely to reach a wide audience. Routine applications of atomic MS are not included in this Update and the reader is referred to the Updates on Industrial Analysis: Metals, Chemicals and Advanced Materials (96/416), Environmental Analysis (96/1444) and Clinical and Biological Materials, Food and Beverages (96/2479). Also excluded are those applications, even if not routine, which use atomic spectroscopy as a tool for the study of a non-atomic property, for example, the use of stable isotope labeling of carbon or nitrogen in biomolecules in metabolic studies. There have been few general reviews on atomic MS of note in the period covered by this update. That of Colodner et al.(95/3890) gave a general review of ion sources, in particular GDMS, ICP-MS, SIMS and TIMS, and that of Blades (95/2568 and 95/3077) was a very general overview of some of the techniques covered in this Update. The review of the literature in the period covered by this Update reveals strong advances in all areas, with a continuing push to achieve better analyses on smaller samples and in less time. Most advances generally require more sophisticated instrumentation, improved sample preparation methods or new methods of sample introduction. This is typified by advances in ICP-MS, which see considerable emphasis on sample introduction techniques and a move towards magnetic sector instruments. Most applications of ICP-MS are now highly routine. There is still, however, a desire to achieve affordable analysis with simplified and cost-effective instruments, as illustrated by the development of mobile, in-situ isotope MS for environmental studies.« less

  12. Cold nuclear fusion

    NASA Astrophysics Data System (ADS)

    Tsyganov, E. N.; Bavizhev, M. D.; Buryakov, M. G.; Dabagov, S. B.; Golovatyuk, V. M.; Lobastov, S. P.

    2015-07-01

    If target deuterium atoms were implanted in a metal crystal in accelerator experiments, a sharp increase in the probability of DD-fusion reaction was clearly observed when compared with the reaction's theoretical value. The electronic screening potential, which for a collision of free deuterium atoms is about 27 eV, reached 300-700 eV in the case of the DD-fusion in metallic crystals. These data leads to the conclusion that a ban must exist for deuterium atoms to be in the ground state 1s in a niche filled with free conduction electrons. At the same time, the state 2p whose energy level is only 10 eV above that of state 1s is allowed in these conditions. With anisotropy of 2p, 3p or above orbitals, their spatial positions are strictly determined in the lattice coordinate system. When filling out the same potential niches with two deuterium atoms in the states 2p, 3p or higher, the nuclei of these atoms can be permanently positioned without creating much Coulomb repulsion at a very short distance from each other. In this case, the transparency of the potential barrier increases dramatically compared to the ground state 1s for these atoms. The probability of the deuterium nuclei penetrating the Coulomb barrier by zero quantum vibration of the DD-system also increases dramatically. The so-called cold nuclear DD-fusion for a number of years was registered in many experiments, however, was still rejected by mainstream science for allegedly having no consistent scientific explanation. Finally, it received the validation. Below, we outline the concept of this explanation and give the necessary calculations. This paper also considers the further destiny of the formed intermediate state of 4He∗.

  13. Adaptive segmentation of nuclei in H&S stained tendon microscopy

    NASA Astrophysics Data System (ADS)

    Chuang, Bo-I.; Wu, Po-Ting; Hsu, Jian-Han; Jou, I.-Ming; Su, Fong-Chin; Sun, Yung-Nien

    2015-12-01

    Tendiopathy is a popular clinical issue in recent years. In most cases like trigger finger or tennis elbow, the pathology change can be observed under H and E stained tendon microscopy. However, the qualitative analysis is too subjective and thus the results heavily depend on the observers. We develop an automatic segmentation procedure which segments and counts the nuclei in H and E stained tendon microscopy fast and precisely. This procedure first determines the complexity of images and then segments the nuclei from the image. For the complex images, the proposed method adopts sampling-based thresholding to segment the nuclei. While for the simple images, the Laplacian-based thresholding is employed to re-segment the nuclei more accurately. In the experiments, the proposed method is compared with the experts outlined results. The nuclei number of proposed method is closed to the experts counted, and the processing time of proposed method is much faster than the experts'.

  14. Method and apparatus for transmutation of atomic nuclei

    DOEpatents

    Maenchen, J.E.; Ruiz, C.L.

    1998-12-08

    Insuring a constant supply of radioisotopes is of great importance to medicine and industry. This invention addresses this problem, and helps to solve it by introducing a new apparatus for transmutation of isotopes which enables swift and flexible production on demand. 9 figs.

  15. Method and apparatus for transmutation of atomic nuclei

    DOEpatents

    Maenchen, J.E.; Ruiz, C.L.

    1998-06-09

    Insuring a constant supply of radioisotopes is of great importance to medicine and industry. This invention addresses this problem, and helps to solve it by introducing a new apparatus for transmutation of isotopes which enables swift and flexible production on demand. 9 figs.

  16. Doubly magic nuclei from lattice QCD forces at MPS=469 MeV /c2

    NASA Astrophysics Data System (ADS)

    McIlroy, C.; Barbieri, C.; Inoue, T.; Doi, T.; Hatsuda, T.

    2018-02-01

    We perform ab initio self-consistent Green's function calculations of the closed shell nuclei 4He, 16O, and 40Ca, based on two-nucleon potentials derived from lattice QCD simulations, in the flavor SU(3) limit and at the pseudoscalar meson mass of 469 MeV/c2. The nucleon-nucleon interaction is obtained using the hadrons-to-atomic-nuclei-from-lattice (HAL) QCD method, and its short-distance repulsion is treated by means of ladder resummations outside the model space. Our results show that this approach diagonalizes ultraviolet degrees of freedom correctly. Therefore, ground-state energies can be obtained from infrared extrapolations even for the relatively hard potentials of HAL QCD. Comparing to previous Brueckner Hartree-Fock calculations, the total binding energies are sensibly improved by the full account of many-body correlations. The results suggest an interesting possible behavior in which nuclei are unbound at very large pion masses and islands of stability appear at first around the traditional doubly magic numbers when the pion mass is lowered toward its physical value. The calculated one-nucleon spectral distributions are qualitatively close to those of real nuclei even for the pseudoscalar meson mass considered here.

  17. Nucleation in Sheared Granular Matter

    NASA Astrophysics Data System (ADS)

    Rietz, Frank; Radin, Charles; Swinney, Harry L.; Schröter, Matthias

    2018-02-01

    We present an experiment on crystallization of packings of macroscopic granular spheres. This system is often considered to be a model for thermally driven atomic or colloidal systems. Cyclically shearing a packing of frictional spheres, we observe a first order phase transition from a disordered to an ordered state. The ordered state consists of crystallites of mixed fcc and hcp symmetry that coexist with the amorphous bulk. The transition, initiated by homogeneous nucleation, overcomes a barrier at 64.5% volume fraction. Nucleation consists predominantly of the dissolving of small nuclei and the growth of nuclei that have reached a critical size of about ten spheres.

  18. Parity and Time-Reversal Violation in Atomic Systems

    NASA Astrophysics Data System (ADS)

    Roberts, B. M.; Dzuba, V. A.; Flambaum, V. V.

    2015-10-01

    Studying the violation of parity and time-reversal invariance in atomic systems has proven to be a very effective means of testing the electroweak theory at low energy and searching for physics beyond it. Recent developments in both atomic theory and experimental methods have led to the ability to make extremely precise theoretical calculations and experimental measurements of these effects. Such studies are complementary to direct high-energy searches, and can be performed for only a fraction of the cost. We review the recent progress in the field of parity and time-reversal violation in atoms, molecules, and nuclei, and examine the implications for physics beyond the Standard Model, with an emphasis on possible areas for development in the near future.

  19. Nucleation of the diamond phase in aluminium-solid solutions

    NASA Technical Reports Server (NTRS)

    Hornbogen, E.; Mukhopadhyay, A. K.; Starke, E. A., Jr.

    1993-01-01

    Precipitation was studied from fcc solid solutions with silicon, germanium, copper and magnesium. Of all these elements only silicon and germanium form diamond cubic (DC) precipitates in fcc Al. Nucleation of the DC structure is enhanced if both types of atom are dissolved in the fcc lattice. This is interpreted as due to atomic size effects in the prenucleation stage. There are two modes of interference of fourth elements with nucleation of the DC phase in Al + Si, Ge. The formation of the DC phase is hardly affected if the atoms (for example, copper) are rejected from the (Si, Ge)-rich clusters. If additional types of atom are attracted by silicon and/or germanium, DC nuclei are replaced by intermetallic compounds (for example Mg2Si).

  20. How large are nonadiabatic effects in atomic and diatomic systems?

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yang, Yubo, E-mail: yyang173@illinois.edu, E-mail: normantubman2015@u.northwestern.edu; Tubman, Norm M., E-mail: yyang173@illinois.edu, E-mail: normantubman2015@u.northwestern.edu; Ceperley, David M.

    2015-09-28

    With recent developments in simulating nonadiabatic systems to high accuracy, it has become possible to determine how much energy is attributed to nuclear quantum effects beyond zero-point energy. In this work, we calculate the non-relativistic ground-state energies of atomic and molecular systems without the Born-Oppenheimer approximation. For this purpose, we utilize the fixed-node diffusion Monte Carlo method, in which the nodes depend on both the electronic and ionic positions. We report ground-state energies for all systems studied, ionization energies for the first-row atoms and atomization energies for the first-row hydrides. We find the ionization energies of the atoms to bemore » nearly independent of the Born-Oppenheimer approximation, within the accuracy of our results. The atomization energies of molecular systems, however, show small effects of the nonadiabatic coupling between electrons and nuclei.« less

  1. How large are nonadiabatic effects in atomic and diatomic systems?

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yang, Yubo; Kylänpää, Ilkka; Tubman, Norm M.

    2015-09-29

    With recent developments in simulating nonadiabatic systems to high accuracy, it has become possible to determine how much energy is attributed to nuclear quantum effects beyond zero-point energy. Here, we calculate the non-relativistic ground-state energies of atomic and molecular systems without the Born-Oppenheimer approximation. For this purpose, we utilize the fixed-node diffusion Monte Carlo method, in which the nodes depend on both the electronic and ionic positions. Our report shows the ground-state energies for all systems studied, ionization energies for the first-row atoms and atomization energies for the first-row hydrides. We find the ionization energies of the atoms to bemore » nearly independent of the Born-Oppenheimer approximation, within the accuracy of our results. The atomization energies of molecular systems, however, show small effects of the nonadiabatic coupling between electrons and nuclei.« less

  2. NMR spectra of androstane analogs of brassinosteroids

    NASA Astrophysics Data System (ADS)

    Baranovskii, A. V.; Litvinovskaya, R. P.; Aver'kova, M. A.; Khripach, N. B.; Khripach, V. A.

    2007-09-01

    We have used two-dimensional NMR spectroscopy to make a complete assignment of signals from the nuclei of hydrogen and carbon atoms in the spectra of brassinosteroids in the androstane series. We have confirmed the stereochemistry of the chiral centers and the structure of the molecules. We have studied the effect of the configuration of the 2,3-diol groups in the A ring of the steroids on the chemical shift of adjacent atoms in the 13C and 1H NMR spectra.

  3. Towards high-resolution laser ionization spectroscopy of the heaviest elements in supersonic gas jet expansion

    PubMed Central

    Ferrer, R.; Barzakh, A.; Bastin, B.; Beerwerth, R.; Block, M.; Creemers, P.; Grawe, H.; de Groote, R.; Delahaye, P.; Fléchard, X.; Franchoo, S.; Fritzsche, S.; Gaffney, L. P.; Ghys, L.; Gins, W.; Granados, C.; Heinke, R.; Hijazi, L.; Huyse, M.; Kron, T.; Kudryavtsev, Yu.; Laatiaoui, M.; Lecesne, N.; Loiselet, M.; Lutton, F.; Moore, I. D.; Martínez, Y.; Mogilevskiy, E.; Naubereit, P.; Piot, J.; Raeder, S.; Rothe, S.; Savajols, H.; Sels, S.; Sonnenschein, V.; Thomas, J-C; Traykov, E.; Van Beveren, C.; Van den Bergh, P.; Van Duppen, P.; Wendt, K.; Zadvornaya, A.

    2017-01-01

    Resonant laser ionization and spectroscopy are widely used techniques at radioactive ion beam facilities to produce pure beams of exotic nuclei and measure the shape, size, spin and electromagnetic multipole moments of these nuclei. However, in such measurements it is difficult to combine a high efficiency with a high spectral resolution. Here we demonstrate the on-line application of atomic laser ionization spectroscopy in a supersonic gas jet, a technique suited for high-precision studies of the ground- and isomeric-state properties of nuclei located at the extremes of stability. The technique is characterized in a measurement on actinium isotopes around the N=126 neutron shell closure. A significant improvement in the spectral resolution by more than one order of magnitude is achieved in these experiments without loss in efficiency. PMID:28224987

  4. A new equation of state Based on Nuclear Statistical Equilibrium for Core-Collapse Simulations

    NASA Astrophysics Data System (ADS)

    Furusawa, Shun; Yamada, Shoichi; Sumiyoshi, Kohsuke; Suzuki, Hideyuki

    2012-09-01

    We calculate a new equation of state for baryons at sub-nuclear densities for the use in core-collapse simulations of massive stars. The formulation is the nuclear statistical equilibrium description and the liquid drop approximation of nuclei. The model free energy to minimize is calculated by relativistic mean field theory for nucleons and the mass formula for nuclei with atomic number up to ~ 1000. We have also taken into account the pasta phase. We find that the free energy and other thermodynamical quantities are not very different from those given in the standard EOSs that adopt the single nucleus approximation. On the other hand, the average mass is systematically different, which may have an important effect on the rates of electron captures and coherent neutrino scatterings on nuclei in supernova cores.

  5. Lifetimes of excited states in triaxially deformed 107Tc and 109,111,113Rh

    NASA Astrophysics Data System (ADS)

    Hagen, T. W.; Görgen, A.; Korten, W.; Grente, L.; Salsac, M.-D.; Farget, F.; Braunroth, T.; Bruyneel, B.; Celikovic, I.; Clément, E.; de France, G.; Delaune, O.; Dewald, A.; Dijon, A.; Hackstein, M.; Jacquot, B.; Litzinger, J.; Ljungvall, J.; Louchart, C.; Michelagnoli, C.; Napoli, D. R.; Recchia, F.; Rother, W.; Sahin, E.; Siem, S.; Sulignano, B.; Theisen, Ch.; Valiente-Dobon, J. J.

    2018-03-01

    Lifetimes of excited states in 107Tc, 109Rh, 111Rh, and 113Rh were measured at GANIL using the Recoil-Distance Doppler Shift method. The neutron-rich nuclei were produced in fission reactions in inverse kinematics with a 238U beam impinging on a 9Be target. Fission fragments were identified event-by-event in the ray-tracing spectrometer VAMOS++ and correlated with prompt γ rays observed around the target position with the EXOGAM Ge detector array. Several lifetimes were obtained for states in the positive-parity yrast bands in the four nuclei and compared to triaxial particle-rotor calculations. The results clarify the configuration for the strongest positive-parity band in 107Tc and suggest a gradual increase of triaxial deformation with atomic number Z, reaching almost maximum triaxiality for the neutron-rich Rh nuclei.

  6. A New Accelerator-Based Mass Spectrometry.

    ERIC Educational Resources Information Center

    Gove, H. E.

    1983-01-01

    Tandem electrostatic accelerators produce beams of positive ions which are used to penetrate atomic nuclei in a target, inducing nuclear reactions whose study elucidates varied properties of the nucleus. Uses of the system, which acts like a mass spectrometer, are discussed. These include radiocarbon dating measurements. (JN)

  7. 11.2 Solar Neutrinos

    NASA Astrophysics Data System (ADS)

    Nakahata, Masayuki

    This document is part of Subvolume A `Theory and Experiments' of Volume 21 `Elementary Particles' of Landolt-Börnstein - Group I `Elementary Particles, Nuclei and Atoms'. It contains of the Chapter `11 Experimental Results on Neutrino Masses and Mixings' the Section `11.2 Solar Neutrinos' with the content:

  8. Nuclear Quantum Effects in Water at the Triple Point: Using Theory as a Link Between Experiments.

    PubMed

    Cheng, Bingqing; Behler, Jörg; Ceriotti, Michele

    2016-06-16

    One of the most prominent consequences of the quantum nature of light atomic nuclei is that their kinetic energy does not follow a Maxwell-Boltzmann distribution. Deep inelastic neutron scattering (DINS) experiments can measure this effect. Thus, the nuclear quantum kinetic energy can be probed directly in both ordered and disordered samples. However, the relation between the quantum kinetic energy and the atomic environment is a very indirect one, and cross-validation with theoretical modeling is therefore urgently needed. Here, we use state of the art path integral molecular dynamics techniques to compute the kinetic energy of hydrogen and oxygen nuclei in liquid, solid, and gas-phase water close to the triple point, comparing three different interatomic potentials and validating our results against equilibrium isotope fractionation measurements. We will then show how accurate simulations can draw a link between extremely precise fractionation experiments and DINS, therefore establishing a reliable benchmark for future measurements and providing key insights to increase further the accuracy of interatomic potentials for water.

  9. Molecular processes in astrophysics: Calculations of hydrogen + hydrogen gas excitation, de-excitation, and cooling

    NASA Astrophysics Data System (ADS)

    Kelley, Matthew Thomas

    The implications of H+H2 cooling in astrophysics is important to several applications. One of the most significant and pure applications is its role in cooling in the early universe. Other applications would include molecular dynamics in nebulae and their collapse into stars and astrophysical shocks. Shortly after the big bang, the universe was a hot primordial gas of photons, electrons, and nuclei among other ingredients. By far the most dominant nuclei in the early universe was hydrogen. In fact, in the early universe the matter density was 90 percent hydrogen and only 10 percent helium with small amounts of lithium and deuterium. In order for structure to form in the universe, this primordial gas must form atoms and cool. One of the significant cooling mechanisms is the collision of neutral atomic hydrogen with a neutral diatomic hydrogen molecule. This work performs calculations to determine collisional cooling rates of hydrogen using two potential surfaces.

  10. Coherent Patterns in Nuclei and in Financial Markets

    NASA Astrophysics Data System (ADS)

    DroŻdŻ, S.; Kwapień, J.; Speth, J.

    2010-07-01

    In the area of traditional physics the atomic nucleus belongs to the most complex systems. It involves essentially all elements that characterize complexity including the most distinctive one whose essence is a permanent coexistence of coherent patterns and of randomness. From a more interdisciplinary perspective, these are the financial markets that represent an extreme complexity. Here, based on the matrix formalism, we set some parallels between several characteristics of complexity in the above two systems. We, in particular, refer to the concept—historically originating from nuclear physics considerations—of the random matrix theory and demonstrate its utility in quantifying characteristics of the coexistence of chaos and collectivity also for the financial markets. In this later case we show examples that illustrate mapping of the matrix formulation into the concepts originating from the graph theory. Finally, attention is drawn to some novel aspects of the financial coherence which opens room for speculation if analogous effects can be detected in the atomic nuclei or in other strongly interacting Fermi systems.

  11. Production of twin /Λ-hypernuclei from Ξ- hyperon capture at rest

    NASA Astrophysics Data System (ADS)

    Ichikawa, A.; Ahn, J. K.; Akikawa, H.; Aoki, S.; Arai, K.; Bahk, S. Y.; Baik, K. M.; Bassalleck, B.; Chung, J. H.; Chung, M. S.; Hoshino, K.; Ieiri, M.; Imai, K.; Iwata, Y. H.; Iwata, Y. S.; Kanda, H.; Kaneko, M.; Kawai, T.; Kim, C. O.; Kim, J. Y.; Kim, S. J.; Kim, S. H.; Kondo, Y.; Kouketsu, T.; Lee, Y. L.; McNabb, J. W. C.; Mitsuhara, M.; Nagase, Y.; Nagoshi, C.; Nakazawa, K.; Noumi, H.; Ogawa, S.; Okabe, H.; Oyama, K.; Park, H. M.; Park, I. G.; Parker, J.; Ra, Y. S.; Rhee, J. T.; Rusek, A.; Shibuya, H.; Sim, K. S.; Saha, P. K.; Seki, D.; Sekimoto, M.; Song, J. S.; Takahashi, H.; Takahashi, T.; Takeutchi, F.; Tanaka, H.; Tanida, K.; Tojo, J.; Torii, H.; Torikai, S.; Ushida, N.; Yamamoto, K.; Yasuda, N.; Yang, J. T.; Yoon, C. J.; Yoon, C. S.; Yosoi, M.; Yoshida, T.; Zhu, L.

    2001-02-01

    A hybrid emulsion experiment was carried out to study double-strangeness nuclei produced via Ξ- hyperon capture at rest with the expectation of ten times larger statistics than previous experiments. We have analyzed 5% of the total emulsion and found one ``twin-hypernuclei'' event involving the emission of two single-/Λ hypernuclei and a nuclear fragment from a Ξ- hyperon stopping point. The event is interpreted as the decay of a Ξ-+14N atomic system to 5ΛHe+5ΛHe+4He+neutron. The species of the Ξ--atom and the fragmentation products are uniquely identified for the first time for twin-hypernuclei events. Combined with the results from a past hybrid-emulsion experiment, one double-/Λ hypernucleus and three twin-hypernuclei events have been found from Ξ- captures on light emulsion nuclei. The ratio of the detected rate of double-/Λ hypernuclei to that of twin-hypernuclei is compared with theoretical estimates.

  12. Space shuttle exhaust cloud properties

    NASA Technical Reports Server (NTRS)

    Anderson, B. J.; Keller, V. W.

    1983-01-01

    A data base describing the properties of the exhaust cloud produced by the launch of the Space Transportation System and the acidic fallout observed after each of the first four launches was assembled from a series of ground and aircraft based measurements made during the launches of STS 2, 3, and 4. Additional data were obtained from ground-based measurements during firings of the 6.4 percent model of the Solid Rocket Booster at the Marshall Center. Analysis indicates that the acidic fallout is produced by atomization of the deluge water spray by the rocket exhaust on the pad followed by rapid scavening of hydrogen chloride gas aluminum oxide particles from the Solid Rocket Boosters. The atomized spray is carried aloft by updrafts created by the hot exhaust and deposited down wind. Aircraft measurements in the STS-3 ground cloud showed an insignificant number of ice nuclei. Although no measurements were made in the column cloud, the possibility of inadvertent weather modification caused by the interaction of ice nuclei with natural clouds appears remote.

  13. Nickel-63 production in copper samples exposed to the Hiroshima atomic bomb: estimation based on an excitation function obtained by neutron irradiation experiments.

    PubMed

    Takamiya, K; Imanaka, T; Ota, Y; Akamine, M; Shibata, S; Shibata, T; Ito, Y; Imamura, M; Uwamino, Y; Nogawa, N; Baba, M; Iwasaki, S; Matsuyama, S

    2008-07-01

    The upper and lower limits of the excitation function of the (63)Cu(n,p)(63)Ni reaction were experimentally determined, and the number of (63)Ni nuclei produced in copper samples exposed to atomic bomb neutrons in Hiroshima was estimated by using the experimental excitation functions and the neutron fluences given in the DS02 dosimetry system. The estimated number of (63)Ni nuclei was compared with that measured and with that calculated using the DS02 dosimetry system and the corresponding ENDF/B-VI cross section. In comparison with DS02, there is about a 60% maximum difference in (63)Ni production at the hypocenter when the experimental upper cross section values are used. The difference becomes smaller at greater distances from the hypocenter and decreases, for example, to less than 30 and 5% when using the upper and lower experimental cross sections at 1,000 m, respectively.

  14. Development of methods for calculating basic features of the nuclear contribution to single event upsets under the effect of protons of moderately high energy

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Chechenin, N. G., E-mail: chechenin@sinp.msu.ru; Chuvilskaya, T. V.; Shirokova, A. A.

    2015-10-15

    As a continuation and a development of previous studies of our group that were devoted to the investigation of nuclear reactions induced by protons of moderately high energy (between 10 and 400 MeV) in silicon, aluminum, and tungsten atoms, the results obtained by exploring nuclear reactions on atoms of copper, which is among the most important components in materials for contact pads and pathways in modern and future ultralarge-scale integration circuits, especially in three-dimensional topology, are reported in the present article. The nuclear reactions in question lead to the formation of the mass and charge spectra of recoil nuclei rangingmore » fromheavy target nuclei down to helium and hydrogen. The kineticenergy spectra of reaction products are calculated. The results of the calculations based on the procedure developed by our group are compared with the results of calculations and experiments performed by other authors.« less

  15. Quantum Chemical Topology: Knowledgeable atoms in peptides

    NASA Astrophysics Data System (ADS)

    Popelier, Paul L. A.

    2012-06-01

    The need to improve atomistic biomolecular force fields remains acute. Fortunately, the abundance of contemporary computing power enables an overhaul of the architecture of current force fields, which typically base their electrostatics on fixed atomic partial charges. We discuss the principles behind the electrostatics of a more realistic force field under construction, called QCTFF. At the heart of QCTFF lies the so-called topological atom, which is a malleable box, whose shape and electrostatics changes in response to a changing environment. This response is captured by a machine learning method called Kriging. Kriging directly predicts each multipole moment of a given atom (i.e. the output) from the coordinates of the nuclei surrounding this atom (i.e. the input). This procedure yields accurate interatomic electrostatic energies, which form the basis for future-proof progress in force field design.

  16. Weizsäcker-Skyrme-type nuclear mass formula incorporating two combinatorial radial basis function prescriptions and their application

    NASA Astrophysics Data System (ADS)

    Ma, Na Na; Zhang, Hai Fei; Yin, Peng; Bao, Xiao Jun; Zhang, Hong Fei

    2017-08-01

    Within the improved Weizsäcker-Skyrme (WS)-type nuclear mass formulas, we systematically calculated one-nucleon and two-nucleon separated energy, α-decay and β-decay energies, and the odd-even staggering (OES) of nuclear binding energies. As a result, the root-mean-square (rms) deviations of 2267 nuclei within the new improved WS-type mass formula are dropped from 493 to 167 keV, where 2267 nuclei are extracted from the atomic mass evaluation of 2012. Simultaneously, all the rms deviations of one-nucleon and two-nucleon separation energies and decay energies Qα,Qβ-,Qβ+, and QEC for more than 3000 nuclei are cut down by about 100-400 keV. Further, some basic physical observations of 988 boundary nuclei are predicted for providing reference to experiments. Finally, the overall neutron OESs and proton OESs have been systemically investigated and the residual error satisfies a normal distribution. The pairing gaps Δn and Δp of the isotopes of O, Ca, Ni, Zr, Sn, Gd, Qs, Pb, Pa, Ds and the isotonic magic chains of N =28 ,50 ,82 ,126 and even-even nuclei are also studied with dramatic improvements obtained. Especially, the rms of Δn and Δp in these nuclei have been reduced by about 200 keV. The above physical quantities show important information for nuclear charts and the features of nuclear structure.

  17. Atomic and Molecular Data and their Applications★

    NASA Astrophysics Data System (ADS)

    Drake, Gordon W. F.; Yoon, Jung-Sik; Kato, Daiji; Karwasz, Grzegorz

    2018-03-01

    This topical issue on Atomic and molecular data and their applications was motivated by the 10th International Conference on Atomic and Molecular Data (ICAMDATA 2016), which was held from September 26 to 29, 2016 in Gunsan, Republic of Korea. The topics of this issue reflect those of the conference program. The scientific papers in the topical issue cover the fields of atomic and molecular structure, radiative transitions, scattering processes, data base development, and the applications of atomic and molecular data to plasma modeling. Contribution to the Topical Issue "Atomic and Molecular Data and their Applications", edited by Gordon W.F. Drake, Jung-Sik Yoon, Daiji Kato, and Grzegorz Karwasz.

  18. Material Science

    NASA Image and Video Library

    2003-02-09

    Materials with a smaller mean atomic mass, such as lithium (Li) hydride and polyethylene, make the best radiation shields for astronauts. The materials have a higher density of nuclei and are better able to block incoming radiation. Also, they tend to produce fewer and less dangerous secondary particles after impact with incoming radiation.

  19. The Gibbs free energy of homogeneous nucleation: From atomistic nuclei to the planar limit.

    PubMed

    Cheng, Bingqing; Tribello, Gareth A; Ceriotti, Michele

    2017-09-14

    In this paper we discuss how the information contained in atomistic simulations of homogeneous nucleation should be used when fitting the parameters in macroscopic nucleation models. We show how the number of solid and liquid atoms in such simulations can be determined unambiguously by using a Gibbs dividing surface and how the free energy as a function of the number of solid atoms in the nucleus can thus be extracted. We then show that the parameters (the chemical potential, the interfacial free energy, and a Tolman correction) of a model based on classical nucleation theory can be fitted using the information contained in these free-energy profiles but that the parameters in such models are highly correlated. This correlation is unfortunate as it ensures that small errors in the computed free energy surface can give rise to large errors in the extrapolated properties of the fitted model. To resolve this problem we thus propose a method for fitting macroscopic nucleation models that uses simulations of planar interfaces and simulations of three-dimensional nuclei in tandem. We show that when the chemical potentials and the interface energy are pinned to their planar-interface values, more precise estimates for the Tolman length are obtained. Extrapolating the free energy profile obtained from small simulation boxes to larger nuclei is thus more reliable.

  20. Preliminary results for salt aerosol production intended for marine cloud brightening, using effervescent spray atomization

    PubMed Central

    Cooper, Gary; Foster, Jack; Galbraith, Lee; Jain, Sudhanshu; Neukermans, Armand; Ormond, Bob

    2014-01-01

    The large-scale production of vast numbers of suitable salt nuclei and their upward launch is one of the main technological barriers to the experimental testing of marine cloud brightening (MCB). Very promising, though not definitive, results have been obtained using an adapted version of effervescent spray atomization. The process is simple, robust and inexpensive. This form of effervescent spraying uses only pressurized water and air sprayed from small nozzles to obtain very fine distributions. While it is far from optimized, and may not be the best method if full deployment is ever desired, we believe that even in its present form the process would lend itself well to preliminary field test investigations of MCB. Measurements obtained using standard aerosol instrumentation show approximately lognormal distributions of salt nuclei with median diameters of approximately 65 nm and geometric standard deviations slightly less than 2. However, these measurements are not in agreement with those based on scanning electron microscopy imaging of collected particles, an observation that has not yet been explained. Assuming the above distribution, 1015 particles per second could be made with 21 kW of spray power, using approximately 200 nozzles. It is envisioned that existing snow making equipment can be adapted to launch the nuclei 60–100 m into the air, requiring approximately 20 kW of additional power. PMID:25404673

  1. Star formation around active galactic nuclei

    NASA Technical Reports Server (NTRS)

    Keel, William C.

    1987-01-01

    Active galactic nuclei (Seyfert nuclei and their relatives) and intense star formation can both deliver substantial amounts of energy to the vicinity of a galactic nucleus. Many luminous nuclei have energetics dominated by one of these mechanisms, but detailed observations show that some have a mixture. Seeing both phenomena at once raises several interesting questions: (1) Is this a general property of some kinds of nuclei? How many AGNs have surround starbursts, and vice versa? (2) As in 1, how many undiscovered AGNs or starbursts are hidden by a more luminous instance of the other? (3) Does one cause the other, and by what means, or do both reflect common influences such as potential well shape or level of gas flow? (4) Can surrounding star formation tell us anything about the central active nuclei, such as lifetimes, kinetic energy output, or mechanical disturbance of the ISM? These are important points in the understanding of activity and star formation in galactic nuclei. Unfortunately, the observational ways of addressing them are as yet not well formulated. Some preliminary studies are reported, aimed at clarifying the issues involved in study of the relationships between stellar and nonstellar excitement in galactic nuclei.

  2. A computational NMR study on zigzag aluminum nitride nanotubes

    NASA Astrophysics Data System (ADS)

    Bodaghi, Ali; Mirzaei, Mahmoud; Seif, Ahmad; Giahi, Masoud

    2008-12-01

    A computational nuclear magnetic resonance (NMR) study is performed to investigate the electronic structure properties of the single-walled zigzag aluminum nitride nanotubes (AlNNTs). The chemical-shielding (CS) tensors are calculated at the sites of Al-27 and N-15 nuclei in three structural forms of AlNNT including H-saturated, Al-terminated, and N-terminated ones. The structural forms are firstly optimized and then the calculated CS tensors in the optimized structures are converted to chemical-shielding isotropic (CSI) and chemical-shielding anisotropic (CSA) parameters. The calculated parameters reveal that various Al-27 and N-15 nuclei are divided into some layers with equivalent electrostatic properties; furthermore, Al and N can act as Lewis base and acid, respectively. In the Al-terminated and N-terminated forms of AlNNT, in which one mouth of the nanotube is terminated by aluminum and nitrogen nuclei, respectively, just the CS tensors of the nearest nuclei to the mouth of the nanotube are significantly changed due to removal of saturating hydrogen atoms. Density functional theory (DFT) calculations are performed using GAUSSIAN 98 package of program.

  3. First lattice QCD study of the gluonic structure of light nuclei

    NASA Astrophysics Data System (ADS)

    Winter, Frank; Detmold, William; Gambhir, Arjun S.; Orginos, Kostas; Savage, Martin J.; Shanahan, Phiala E.; Wagman, Michael L.; Nplqcd Collaboration

    2017-11-01

    The role of gluons in the structure of the nucleon and light nuclei is investigated using lattice quantum chromodynamics (QCD) calculations. The first moment of the unpolarized gluon distribution is studied in nuclei up to atomic number A =3 at quark masses corresponding to pion masses of mπ˜450 and 806 MeV. Nuclear modification of this quantity defines a gluonic analogue of the EMC effect and is constrained to be less than ˜10 % in these nuclei. This is consistent with expectations from phenomenological quark distributions and the momentum sum rule. In the deuteron, the combination of gluon distributions corresponding to the b1 structure function is found to have a small first moment compared with the corresponding momentum fraction. The first moment of the gluon transversity structure function is also investigated in the spin-1 deuteron, where a nonzero signal is observed at mπ˜806 MeV . This is the first indication of gluon contributions to nuclear structure that can not be associated with an individual nucleon.

  4. First lattice QCD study of the gluonic structure of light nuclei

    DOE PAGES

    Winter, Frank; Detmold, William; Gambhir, Arjun S.; ...

    2017-11-28

    The role of gluons in the structure of the nucleon and light nuclei is investigated using lattice quantum chromodynamics (QCD) calculations. The first moment of the unpolarised gluon distribution is studied in nuclei up to atomic numbermore » $A=3$ at quark masses corresponding to pion masses of $$m_\\pi\\sim 450$$ and $806$ MeV. Nuclear modification of this quantity defines a gluonic analogue of the EMC effect and is constrained to be less than $$\\sim 10$$% in these nuclei. This is consistent with expectations from phenomenological quark distributions and the momentum sum rule. In the deuteron, the combination of gluon distributions corresponding to the $$b_1$$ structure function is found to have a small first moment compared with the corresponding momentum fraction. The first moment of the gluon transversity structure function is also investigated in the spin-1 deuteron, where a non-zero signal is observed at $$m_\\pi \\sim 806$$ MeV. In conclusion, this is the first indication of gluon contributions to nuclear structure that can not be associated with an individual nucleon.« less

  5. An Adaptive QSE-reduced Nuclear Reaction Network for Silicon Burning

    NASA Astrophysics Data System (ADS)

    Parete-Koon, Suzanne; Hix, William Raphael; Thielemann, Friedrich-Karl

    2010-02-01

    The nuclei of the ``iron peak'' are formed late in the evolution of massive stars and during supernovae. Silicon burning during these events is responsible for the production of a wide range of nuclei with atomic mass numbers from 28 to 64. The large number of nuclei involved make accurate modeling of silicon burning computationally expensive. Examination of the physics of silicon burning reveals that the nuclear evolution is dominated by large groups of nuclei in mutual equilibrium. We present an improvement on our hybrid equilibrium-network scheme that takes advantage of this quasi-equilibrium (QSE) to reduce the number of independent variables calculated. Because the membership and number of these groups vary as the temperature, density and electron faction change, achieving maximal efficiency requires dynamic adjustment of group number and membership. The resultant QSE-reduced network is up to 20 times faster than the full network it replaces without significant loss of accuracy. These reductions in computational cost and the number of species evolved make QSE-reduced networks well suited for inclusion within hydrodynamic simulations, particularly in multi-dimensional applications. )

  6. A new baryonic equation of state at sub-nuclear densities for core-collapse simulations

    NASA Astrophysics Data System (ADS)

    Furusawa, Shun; Yamada, Shoichi; Sumiyoshi, Kohsuke; Suzuki, Hideyuki

    2012-11-01

    We construct a new equation of state for baryons at sub-nuclear densities for the use in core-collapse simulations of massive stars. The formulation is based on the nuclear statistical equilibrium description and the liquid drop approximation of nuclei. The model free energy to minimize is calculated by using relativistic mean field theory for nucleons and the mass formula for nuclei with atomic number up to ~ 1000. We have also taken into account the pasta phase. We find that the free energy and other thermodynamical quantities are not very different from those given in the standard EOSs that adopt the single nucleus approximation. On the other hand, the average mass is systematically different, which may have an important effect to the rates of electron captures and coherent neutrino scatterings on nuclei in supernova cores. It is also interesting that the root mean square of the mass number is not very different from the average mass number, since the former is important for the evaluation of coherent scattering rates on nuclei but has been unavailable so far.

  7. New, simplified, interpolation method for estimation of microscopic nuclear masses based on the p-factor, P = N/sub P/N/sub N//(N/sub p/+N/sub n/)

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Haustein, P.E.; Brenner, D.S.; Casten, R.F.

    1987-12-10

    A new semi-empirical method, based on the use of the P-factor (P = N/sub p/N/sub n//(N/sub p/+N/sub n/)), is shown to simplify significantly the systematics of atomic masses. Its uses is illustrated for actinide nuclei where complicated patterns of mass systematics seen in traditional plots versus Z, N, or isospin are consolidated and transformed into linear ones extending over long isotopic and isotonic sequences. The linearization of the systematics by this procedure provides a simple basis for mass prediction. For many unmeasured nuclei beyond the known mass surface, the P-factor method operates by interpolation among data for known nuclei rathermore » than by extrapolation, as is common in other mass models.« less

  8. Nuclear inertia and the decay modes of superheavy nuclei

    NASA Astrophysics Data System (ADS)

    Poenaru, D. N.; Gherghescu, R. A.; Greiner, Walter

    2013-10-01

    Superheavy nuclei produced up to now decay mainly by α emission and spontaneous fission. For atomic numbers larger than 121 cluster decay has a good chance to compete. While calculated α decay half-lives are in agreement with experimental data within one order of magnitude and cluster decay experiments are also very well accounted for, the discrepancy between theory and experiment can be as high as ten orders of magnitude for spontaneous fission. We analyze some ways of improving the accuracy: using a semiempirical formula for α decay and changing the parameters of analytical superasymmetric fission and of the universal curve for cluster decay. For spontaneous fission we act on nuclear dynamics based on potential barriers computed by the macroscopic-microscopic method and employing various nuclear inertia variation laws. Applications are illustrated for 284Cn and Z = 118-124 even-even parent nuclei. Communicated by Steffen Bass

  9. CRPropa 2.0 - A public framework for propagating high energy nuclei, secondary gamma rays and neutrinos

    NASA Astrophysics Data System (ADS)

    Kampert, Karl-Heinz; Kulbartz, Jörg; Maccione, Luca; Nierstenhoefer, Nils; Schiffer, Peter; Sigl, Günter; van Vliet, Arjen René

    2013-02-01

    Version 2.0 of CRPropa [CRPropa is published under the 3rd version of the GNU General Public License (GPLv3). It is available, together with a detailed documentation of the code, at https://crpropa.desy.de.] is public software to model the extra-galactic propagation of ultra-high energy nuclei of atomic number Z⩽26 through structured magnetic fields and ambient photon backgrounds taking into account all relevant particle interactions. CRPropa covers the energy range 7×1016

  10. Statistical Analysis For Nucleus/Nucleus Collisions

    NASA Technical Reports Server (NTRS)

    Mcguire, Stephen C.

    1989-01-01

    Report describes use of several statistical techniques to charactertize angular distributions of secondary particles emitted in collisions of atomic nuclei in energy range of 24 to 61 GeV per nucleon. Purpose of statistical analysis to determine correlations between intensities of emitted particles and angles comfirming existence of quark/gluon plasma.

  11. Students' use of atomic and molecular models in learning chemistry

    NASA Astrophysics Data System (ADS)

    O'Connor, Eileen Ann

    1997-09-01

    The objective of this study was to investigate the development of introductory college chemistry students' use of atomic and molecular models to explain physical and chemical phenomena. The study was conducted during the first semester of the course at a University and College II. Public institution (Carnegie Commission of Higher Education, 1973). Students' use of models was observed during one-on-one interviews conducted over the course of the semester. The approach to introductory chemistry emphasized models. Students were exposed to over two-hundred and fifty atomic and molecular models during lectures, were assigned text readings that used over a thousand models, and worked interactively with dozens of models on the computer. These models illustrated various features of the spatial organization of valence electrons and nuclei in atoms and molecules. Despite extensive exposure to models in lectures, in textbook, and in computer-based activities, the students in the study based their explanation in large part on a simple Bohr model (electrons arranged in concentric circles around the nuclei)--a model that had not been introduced in the course. Students used visual information from their models to construct their explanation, while overlooking inter-atomic and intra-molecular forces which are not represented explicitly in the models. In addition, students often explained phenomena by adding separate information about the topic without either integrating or logically relating this information into a cohesive explanation. The results of the study demonstrate that despite the extensive use of models in chemistry instruction, students do not necessarily apply them appropriately in explaining chemical and physical phenomena. The results of this study suggest that for the power of models as aids to learning to be more fully realized, chemistry professors must give more attention to the selection, use, integration, and limitations of models in their instruction.

  12. Ab initio simulation of particle momentum distributions in high-pressure water

    NASA Astrophysics Data System (ADS)

    Ceriotti, M.

    2014-12-01

    Applying pressure to water reduces the average oxygen-oxygen distance, and facilitates the delocalisation of protons along the hydrogen bond. This pressure-induced delocalisation is further enhanced by the quantum nature of hydrogen nuclei, which is very significant even well above room temperature. Here we will evaluate the quantum kinetic energy and the particle momentum distribution of hydrogen and oxygen nuclei in water at extreme pressure, using ab initio path integral molecular dynamics. We will show that (transient) dissociation of water molecules induce measurable changes in the kinetic energy hydrogen atoms, although current deep inelastic scattering experiments are probably unable to capture the heterogeneity of the sample.

  13. Experimental level densities of atomic nuclei

    DOE PAGES

    Guttormsen, M.; Aiche, M.; Bello Garrote, F. L.; ...

    2015-12-23

    It is almost 80 years since Hans Bethe described the level density as a non-interacting gas of protons and neutrons. In all these years, experimental data were interpreted within this picture of a fermionic gas. However, the renewed interest of measuring level density using various techniques calls for a revision of this description. In particular, the wealth of nuclear level densities measured with the Oslo method favors the constant-temperature level density over the Fermi-gas picture. Furthermore, trom the basis of experimental data, we demonstrate that nuclei exhibit a constant-temperature level density behavior for all mass regions and at least upmore » to the neutron threshold.« less

  14. Hard probes of short-range nucleon-nucleon correlations

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    J. Arrington, D. W. Higinbotham, G. Rosner, M. Sargsian

    2012-10-01

    The strong interaction of nucleons at short distances leads to a high-momentum component to the nuclear wave function, associated with short-range correlations between nucleons. These short-range, high-momentum structures in nuclei are one of the least well understood aspects of nuclear matter, relating to strength outside of the typical mean-field approaches to calculating the structure of nuclei. While it is difficult to study these short-range components, significant progress has been made over the last decade in determining how to cleanly isolate short-range correlations in nuclei. We have moved from asking if such structures exist, to mapping out their strength in nucleimore » and studying their microscopic structure. A combination of several different measurements, made possible by high-luminosity and high-energy accelerators, coupled with an improved understanding of the reaction mechanism issues involved in studying these structures, has led to significant progress, and provided significant new information on the nature of these small, highly-excited structures in nuclei. We review the general issues related to short-range correlations, survey recent experiments aimed at probing these short-range structures, and lay out future possibilities to further these studies.« less

  15. Local order parameters for use in driving homogeneous ice nucleation with all-atom models of water

    NASA Astrophysics Data System (ADS)

    Reinhardt, Aleks; Doye, Jonathan P. K.; Noya, Eva G.; Vega, Carlos

    2012-11-01

    We present a local order parameter based on the standard Steinhardt-Ten Wolde approach that is capable both of tracking and of driving homogeneous ice nucleation in simulations of all-atom models of water. We demonstrate that it is capable of forcing the growth of ice nuclei in supercooled liquid water simulated using the TIP4P/2005 model using over-biassed umbrella sampling Monte Carlo simulations. However, even with such an order parameter, the dynamics of ice growth in deeply supercooled liquid water in all-atom models of water are shown to be very slow, and so the computation of free energy landscapes and nucleation rates remains extremely challenging.

  16. LAD Prize Talk: Lab Astro and the Origins of the Chemical Elements

    NASA Astrophysics Data System (ADS)

    Lawler, James E.

    2017-06-01

    Only a few of the lightest or primordial nuclei were made just after the Big Bang. Other light nuclei up to the Fe-group are made by fusion in stars. Heavier nuclei are made primarily via r(apid)-process and s(low)-process n(eutron)-capture events. Although the s-process n-capture is fairly well understood, the r-process n-capture events remain poorly understood. The relative role of Core Collapse SNe and n-star mergers will likely be understood in the next few decades. I will discuss recent studies of old Metal-Poor stars that are revealing some new details of nucleosynthesis. This progress is due to the availability of high resolution spectra from large ground based telescopes, access to the UV via HST, and better laboratory data. Our laboratory astrophysics program has focused primarily on the measurement of transition probabilities by combining radiative lifetimes with emission branching fractions. The use of Time Resolved Laser Induced Fluorescence (TRLIF) to measure radiative lifetimes in metallic atoms and ions provides an absolute scale for transition probabilities accurate to a few percent [e.g. 1]. The development and application of TRLIF to neutral and ionized atoms of nearly all elements is due to a simple, versatile, and reliable atom/ion beam source based on a hollow cathode discharge [2, 3]. Fourier transform spectrometers (FTSs) are essential in the measurement of emission branching fractions for atoms and ions with dense spectra such as the rare earths [e.g. 4, 5]. A 3 m focal length echelle spectrometer is important to the measurement of weak branches which might otherwise be obscured by multiplex noise in FTS data [6, 7]. References: [1] E. A. Den Hartog et al., ApJS 194: 35 (2011). [2] D. W. Duquette et al., Phys. Rev. A24, 2847 (1981). [3] S. Salih & J. E. Lawler, Phys. Rev. A29, 3753, (1983). [4] J. W. Brault, J. Opt. Soc. Am. 66, 1081 (1976). [5] J. E. Lawler et al., ApJS 182, 51 (2009). [6] M. P. Wood & J. E. Lawler, Appl. Opt. 51, 8407 (2012). [7] C. Sneden et al., ApJ 817:53 (2016).

  17. Architecture of Pd-Au bimetallic nanoparticles in sodium bis(2-ethylhexyl)sulfosuccinate reverse micelles as investigated by X-ray absorption spectroscopy.

    PubMed

    Chen, Ching-Hsiang; Sarma, Loka Subramanyam; Chen, Jium-Ming; Shih, Shou-Chu; Wang, Guo-Rung; Liu, Din-Goa; Tang, Mau-Tsu; Lee, Jyh-Fu; Hwang, Bing-Joe

    2007-09-01

    In this study, we demonstrate the unique application of X-ray absorption spectroscopy (XAS) as a fundamental characterization tool to help in designing and controlling the architecture of Pd-Au bimetallic nanoparticles within a water-in-oil microemulsion system of water/sodium bis(2-ethylhexyl)sulfosuccinate (AOT)/n-heptane. Structural insights obtained from the in situ XAS measurements recorded at each step during the formation process revealed that Pd-Au bimetallic clusters with various Pd-Au atomic stackings are formed by properly performing hydrazine reduction and redox transmetalation reactions sequentially within water-in-oil microemulsions. A structural model is provided to explain reasonably each reaction step and to give detailed insight into the nucleation and growth mechanism of Pd-Au bimetallic clusters. The combination of in situ XAS analysis at both the Pd K-edge and the Au L(III)-edge and UV-vis absorption spectral features confirms that the formation of Pd-Au bimetallic clusters follows a (Pd(nuclei)-Au(stack))-Pd(surf) stacking. This result further implies that the thickness of Au(stack) and Pd(surf) layers may be modulated by varying the dosage of the Au precursor and hydrazine, respectively. In addition, a bimetallic (Pd-Au)(alloy) nanocluster with a (Pd(nuclei)-Au(stack))-(Pd-Au(alloy))(surf) stacking was also designed and synthesized in order to check the feasibility of Pd(surf) layer modification. The result reveals that the Pd(surf) layer of the stacked (Pd(nuclei)-Au)(stack) bimetallic clusters can be successfully modified to form a (Au-Pd alloy)(surf) layer by a co-reduction of Pd and Au ions by hydrazine. Further, we demonstrate the alloying extent or atomic distribution of Pd and Au in Pd-Au bimetallic nanoparticles from the derived XAS structural parameters. The complete XAS-based methodology, demonstrated here on the Pd-Au bimetallic system, can easily be extended to design and control the alloying extent or atomic distribution, atomic stacking, and electronic structure to construct many other types of bimetallic systems for interesting applications.

  18. Studies of Heavy-Ion Reactions and Transuranic Nuclei

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Schroeder, W. Udo

    2016-07-28

    Studies of heavy-ion reactions and transuranic nuclei performed by the University of Rochester Nuclear Science Research Group have been successful in furthering experimental systematics and theoretical understanding of the behavior of nuclear systems excited to their limits of stability. The theoretical results explain specifically the “boiling” and “vaporization” of atomic nuclei, but are more generally applicable to isolated, quantal many-particle systems which, under thermal or mechanical stresses, all disintegrate by evaporation, via surface cluster emission, or via fission-like processes. Accompanying experimental investigations by the group have demonstrated several new types of dynamical instability of nuclei: In central, “head-on” collisions, targetmore » nuclei exhibit limited ability to stop energetic projectile nuclei and to dissipate the imparted linear momentum. Substantial matter overlap (“neck”) between projectile and target nuclei, which is observed at elevated collision energies, can be stretched considerably and break at several places simultaneously. These results provide new testing grounds for microscopic theory of the cohesion of nuclear matter. This property has remained elusive, even though the elementary nucleon-nucleon forces are well known since some time. Technical R&D has resulted in a detailed characterization of a novel plastic material, which can now be used in the design of sensitive diagnostic systems for various types of radio-activity. Innovative application of powerful laser systems has produced intense, controllable sources of exotic particle radioactivity for nuclear investigations. Several students have received their Ph.D. degree in experimental nuclear science for their work on basic nuclear research or R&D projects.« less

  19. William Fowler and Elements in the Stars

    Science.gov Websites

    some of the most central issues in modern physics and cosmology: the formation of the chemical elements . Documents: Energy Levels of Light Nuclei. III; Review of Modern Physics, Vol 22, Issue 4:291-372; October

  20. Physics Division annual report 2004.

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Glover, J.

    2006-04-06

    This report highlights the research performed in 2004 in the Physics Division of Argonne National Laboratory. The Division's programs include operation of ATLAS as a national user facility, nuclear structure and reaction research, nuclear theory, medium energy nuclear research and accelerator research and development. The intellectual challenges of this research represent some of the most fundamental challenges in modern science, shaping our understanding of both tiny objects at the center of the atom and some of the largest structures in the universe. A great strength of these efforts is the critical interplay of theory and experiment. Notable results in researchmore » at ATLAS include a measurement of the charge radius of He-6 in an atom trap and its explanation in ab-initio calculations of nuclear structure. Precise mass measurements on critical waiting point nuclei in the rapid-proton-capture process set the time scale for this important path in nucleosynthesis. An abrupt fall-off was identified in the subbarrier fusion of several heavy-ion systems. ATLAS operated for 5559 hours of research in FY2004 while achieving 96% efficiency of beam delivery for experiments. In Medium Energy Physics, substantial progress was made on a long-term experiment to search for the violation of time-reversal invariance using trapped Ra atoms. New results from HERMES reveal the influence of quark angular momentum. Experiments at JLAB search for evidence of color transparency in rho-meson production and study the EMC effect in helium isotopes. New theoretical results include a Poincare covariant description of baryons as composites of confined quarks and non-point-like diquarks. Green's function Monte Carlo techniques give accurate descriptions of the excited states of light nuclei and these techniques been extended to scattering states for astrophysics studies. A theoretical description of the phenomena of proton radioactivity has been extended to triaxial nuclei. Argonne continues to lead in the development and exploitation of the new technical concepts that will truly make RIA, in the words of NSAC, ''the world-leading facility for research in nuclear structure and nuclear astrophysics''. The performance standards for new classes of superconducting cavities continue to increase. Driver linac transients and faults have been analyzed to understand reliability issues and failure modes. Liquid-lithium targets were shown to successfully survive the full-power deposition of a RIA beam. Our science and our technology continue to point the way to this major advance. It is a tremendously exciting time in science for RIA holds the keys to unlocking important secrets of nature. The work described here shows how far we have come and makes it clear we know the path to meet these intellectual challenges. The great progress that has been made in meeting the exciting intellectual challenges of modern nuclear physics reflects the talents and dedication of the Physics Division staff and the visitors, guests and students who bring so much to the research.« less

  1. Resolving the neutron lifetime puzzle

    NASA Astrophysics Data System (ADS)

    Mumm, Pieter

    2018-05-01

    Free electrons and protons are stable, but outside atomic nuclei, free neutrons decay into a proton, electron, and antineutrino through the weak interaction, with a lifetime of ∼880 s (see the figure). The most precise measurements have stated uncertainties below 1 s (0.1%), but different techniques, although internally consistent, disagree by 4 standard deviations given the quoted uncertainties. Resolving this “neutron lifetime puzzle” has spawned much experimental effort as well as exotic theoretical mechanisms, thus far without a clear explanation. On page 627 of this issue, Pattie et al. (1) present the most precise measurement of the neutron lifetime to date. A new method of measuring trapped neutrons in situ allows a more detailed exploration of one of the more pernicious systematic effects in neutron traps, neutron phase-space evolution (the changing orbits of neutrons in the trap), than do previous methods. The precision achieved, combined with a very different set of systematic uncertainties, gives hope that experiments such as this one can help resolve the current situation with the neutron lifetime.

  2. Penning Trap Experiments with the Most Exotic Nuclei on Earth: Precision Mass Measurements of Halo Nuclei

    NASA Astrophysics Data System (ADS)

    Brodeur, M.; Brunner, T.; Ettenauer, S.; Lapierre, A.; Ringle, R.; Delheij, P.; Dilling, J.

    2009-05-01

    Exotic nuclei are characterized with an extremely unbalanced protons-neutrons ratio (p/n) where for instance, the halo isotopes of He and Li have up to 3X more n than p (compared to p/n = 1 in ^12C). The properties of these exotic halo nuclei have long been recognized as the most stringent tests of our understanding of the strong force. ^11Li belongs to a special category of halos called Borromean, bound as a three-body family, while the two-body siblings, ^10Li and 2 n, are unbound as separate entities. Last year, a first mass measurement of the radioisotope ^11Li using a Penning trap spectrometer was carried out at the TITAN (Triumf's Ion Trap for Atomic and Nuclear science) facility at TRIUMF-ISAC. Penning traps are proven to be the most precise device to make mass measurements, yet until now they were unable to reach these nuclei. At TRIUMF we managed to measure the mass of ^11Li to an unprecedented precision of dm/m = 60 ppb, which is remarkable since it has a half-life of only 8.8 ms which it the shortest-lived nuclide to be measured with this technique. Furthermore, new and improved masses for the 2 and 4 n halo ^6,8He, as well has the 1 n halo ^11Be have been performed. An overview of the TITAN mass measurement program and its impact in understanding the most exotic nuclei will be given.

  3. Nuclear magnetic resonance studies of quadrupolar nuclei and dipolar field effects

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Urban, Jeffry Todd

    Experimental and theoretical research conducted in two areas in the field of nuclear magnetic resonance (NMR) spectroscopy is presented: (1) studies of the coherent quantum-mechanical control of the angular momentum dynamics of quadrupolar (spin I > 1/2) nuclei and its application to the determination of molecular structure; and (2) applications of the long-range nuclear dipolar field to novel NMR detection methodologies.The dissertation is organized into six chapters. The first two chapters and associated appendices are intended to be pedagogical and include an introduction to the quantum mechanical theory of pulsed NMR spectroscopy and the time dependent theory of quantum mechanics.more » The third chapter describes investigations of the solid-state multiple-quantum magic angle spinning (MQMAS) NMR experiment applied to I = 5/2 quadrupolar nuclei. This work reports the use of rotary resonance-matched radiofrequency irradiation for sensitivity enhancement of the I = 5/2 MQMAS experiment. These experiments exhibited certain selective line narrowing effects which were investigated theoretically.The fourth chapter extends the discussion of multiple quantum spectroscopy of quadrupolar nuclei to a mostly theoretical study of the feasibility of enhancing the resolution of nitrogen-14 NMR of large biomolecules in solution via double-quantum spectroscopy. The fifth chapter continues to extend the principles of multiple quantum NMR spectroscopy of quadrupolar nuclei to make analogies between experiments in NMR/nuclear quadrupolar resonance (NQR) and experiments in atomic/molecular optics (AMO). These analogies are made through the Hamiltonian and density operator formalism of angular momentum dynamics in the presence of electric and magnetic fields.The sixth chapter investigates the use of the macroscopic nuclear dipolar field to encode the NMR spectrum of an analyte nucleus indirectly in the magnetization of a sensor nucleus. This technique could potentially serve as an encoding module for the recently developed NMR remote detection experiment. The feasibility of using hyperpolarized xenon-129 gas as a sensor is discussed. This work also reports the use of an optical atomic magnetometer to detect the nuclear magnetization of Xe-129 gas, which has potential applicability as a detection module for NMR remote detection experiments.« less

  4. Nuclear Structure of 186Re

    DTIC Science & Technology

    2016-12-24

    D population-depopulation . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 101 AME Atomic Mass Evaluation...this mass region are important for validating models of nuclear structure and reactions. The ENSDF feeds a specific data library relevant to nuclear...spherically asymmetric. Spherical asymmetry is common for nuclei between shell closures, such as those in the mid-shell 150  A  190 mass range of interest

  5. What Is a Chemical Element?

    ERIC Educational Resources Information Center

    ten Hoor, Marten J.

    2017-01-01

    Contrary to current IUPAC recommendations, the chemical element X should be defined as the nucleus of the X atom. Consequently, different isotopes with their different nuclei belong to different elements, each one with its own physical and chemical properties. This view leads to the conclusion that we no longer have a periodic table of the…

  6. A Geant4-based Simulation to Evaluate the Feasibility of Using Nuclear Resonance Fluorescence (NRF) in Determining Atomic Compositions of Body Tissue in Cancer Diagnostics and Irradiation

    NASA Astrophysics Data System (ADS)

    Gilbo, Yekaterina; Wijesooriya, Krishni; Liyanage, Nilanga

    2017-01-01

    Customarily applied in homeland security for identifying concealed explosives and chemical weapons, NRF (Nuclear Resonance Fluorescence) may have high potential in determining atomic compositions of body tissue. High energy photons incident on a target excite the target nuclei causing characteristic re-emission of resonance photons. As the nuclei of each isotope have well-defined excitation energies, NRF uniquely indicates the isotopic content of the target. NRF radiation corresponding to nuclear isotopes present in the human body is emitted during radiotherapy based on Bremsstrahlung photons generated in a linear electron accelerator. We have developed a Geant4 simulation in order to help assess NRF capabilities in detecting, mapping, and characterizing tumors. We have imported a digital phantom into the simulation using anatomical data linked to known chemical compositions of various tissues. Work is ongoing to implement the University of Virginia's cancer center treatment setup and patient geometry, and to collect and analyze the simulation's physics quantities to evaluate the potential of NRF for medical imaging applications. Preliminary results will be presented.

  7. Towards Single Biomolecule Imaging via Optical Nanoscale Magnetic Resonance Imaging.

    PubMed

    Boretti, Alberto; Rosa, Lorenzo; Castelletto, Stefania

    2015-09-09

    Nuclear magnetic resonance (NMR) spectroscopy is a physical marvel in which electromagnetic radiation is charged and discharged by nuclei in a magnetic field. In conventional NMR, the specific nuclei resonance frequency depends on the strength of the magnetic field and the magnetic properties of the isotope of the atoms. NMR is routinely utilized in clinical tests by converting nuclear spectroscopy in magnetic resonance imaging (MRI) and providing 3D, noninvasive biological imaging. While this technique has revolutionized biomedical science, measuring the magnetic resonance spectrum of single biomolecules is still an intangible aspiration, due to MRI resolution being limited to tens of micrometers. MRI and NMR have, however, recently greatly advanced, with many breakthroughs in nano-NMR and nano-MRI spurred by using spin sensors based on an atomic impurities in diamond. These techniques rely on magnetic dipole-dipole interactions rather than inductive detection. Here, novel nano-MRI methods based on nitrogen vacancy centers in diamond are highlighted, that provide a solution to the imaging of single biomolecules with nanoscale resolution in-vivo and in ambient conditions. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  8. Empirical moments of inertia of axially asymmetric nuclei

    DOE PAGES

    Allmond, J. M.; Wood, J. L.

    2017-02-06

    We extracted empirical moments of inertia, J1, J2, J3, of atomic nuclei with E(4more » $$+\\atop{1}$$)/E(2$$+\\atop{1}$$ ) > 2.7 from experimental 2$$+\\atop{g,y}$$, energies and electric quadrupole matrix elements, determined from multi- step Coulomb excitation data, and the results are compared to expectations based on rigid and irro- tational inertial flow. Only by having the signs of the E2 matrix elements, i.e., <2$$+\\atop{g}$$ ||M (E2)||2$$+\\atop{g}$$> and <0$$+\\atop{g}$$ ||M (E2)||2$$+\\atop{g}$$> < 2$$+\\atop{g}$$ ||M (E2)||2$$+\\atop{γ}$$> <2$$+\\atop{γ}$$ ||M (E2)||0$$+\\atop{g}$$> , can a unique solution to all three components of the inertia tensor of an asymmetric top be obtained. And while the absolute moments of inertia fall between the rigid and irrotational values as expected, the relative moments of inertia appear to be qualitatively consistent with the β 2 sin 2(γ ) dependence of the Bohr Hamiltonian which originates from a SO(5) in- variance. A better understanding of inertial flow is central to improving collective models, particularly hydrodynamic-based collective models. The results suggest that a better description of collective dynamics and inertial flow for atomic nuclei is needed. The inclusion of vorticity degrees of freedom may provide a path forward. This is our first report of empirical moments of inertia for all three axes and the results should challenge both collective and microscopic descriptions of inertial flow.« less

  9. Alpha Decay Potential Barriers and Half-Lives and Analytical Formula Predictions for Superheavy Nuclei

    NASA Astrophysics Data System (ADS)

    Royer, Guy; Zhang, Hongfei

    The α decay potential barriers are determined in the cluster-like shape path within a generalized liquid drop model including the proximity effects between the α particle and the daughter nucleus and adjusted to reproduce the experimental Qα. The α emission half-lives are determined within the WKB penetration probability. Calculations using previously proposed formulae depending only on the mass and charge of the alpha emitter and Qα are also compared with new experimental alpha-decay half-lives. The agreement allows to provide predictions for the α decay half-lives of other still unknown superheavy nuclei using the Qα determined from the 2003 atomic mass evaluation of Audi, Wapstra and Thibault.

  10. The QSE-Reduced Nuclear Reaction Network for Silicon Burning

    NASA Astrophysics Data System (ADS)

    Hix, W. Raphael; Parete-Koon, Suzanne T.; Freiburghaus, Christian; Thielemann, Friedrich-Karl

    2007-09-01

    Iron and neighboring nuclei are formed in massive stars shortly before core collapse and during their supernova outbursts, as well as during thermonuclear supernovae. Complete and incomplete silicon burning are responsible for the production of a wide range of nuclei with atomic mass numbers from 28 to 64. Because of the large number of nuclei involved, accurate modeling of silicon burning is computationally expensive. However, examination of the physics of silicon burning has revealed that the nuclear evolution is dominated by large groups of nuclei in mutual equilibrium. We present a new hybrid equilibrium-network scheme which takes advantage of this quasi-equilibrium in order to reduce the number of independent variables calculated. This allows accurate prediction of the nuclear abundance evolution, deleptonization, and energy generation at a greatly reduced computational cost when compared to a conventional nuclear reaction network. During silicon burning, the resultant QSE-reduced network is approximately an order of magnitude faster than the full network it replaces and requires the tracking of less than a third as many abundance variables, without significant loss of accuracy. These reductions in computational cost and the number of species evolved make QSE-reduced networks well suited for inclusion within hydrodynamic simulations, particularly in multidimensional applications.

  11. Empirical p-n interactions, the synchronized filling of Nilsson orbitals, and emergent collectivity

    NASA Astrophysics Data System (ADS)

    Cakirli, R. B.

    2014-09-01

    The onset of collectivity and deformation, changes to the single particle energies and magic numbers and so on are strongly influenced by, for example, proton (p) and neutron (n) interactions inside atomic nuclei. Experimentally, using binding energies (or masses), one can extract an average p-n interaction between the last two protons and the last two neutrons, called δVpn. We have studied δVpn values using calculations of spatial overlaps between p and n Nilsson orbitals, considering different deformations, for the Z= 50-82, N= 82-126 shells, and comparison of these theoretical results with experimental δVpn values. Our results show that enhanced valence p-n interactions are closely correlated with the development of collectivity, shape changes, and the saturation of deformation in nuclei. We note that the difference of the Nilsson quantum numbers of the last filled Nilsson p and n orbitals, has a special relation, 0[110], in which they differ by only a single quantum in the z-direction, for those nuclei where δVpn is largest for each Z in medium mass and heavy nuclei. The synchronised filling of such orbital pairs correlates with the emergence of collectivity.

  12. Emergent properties of nuclei from ab initio coupled-cluster calculations

    NASA Astrophysics Data System (ADS)

    Hagen, G.; Hjorth-Jensen, M.; Jansen, G. R.; Papenbrock, T.

    2016-06-01

    Emergent properties such as nuclear saturation and deformation, and the effects on shell structure due to the proximity of the scattering continuum and particle decay channels are fascinating phenomena in atomic nuclei. In recent years, ab initio approaches to nuclei have taken the first steps towards tackling the computational challenge of describing these phenomena from Hamiltonians with microscopic degrees of freedom. This endeavor is now possible due to ideas from effective field theories, novel optimization strategies for nuclear interactions, ab initio methods exhibiting a soft scaling with mass number, and ever-increasing computational power. This paper reviews some of the recent accomplishments. We also present new results. The recently optimized chiral interaction NNLO{}{{sat}} is shown to provide an accurate description of both charge radii and binding energies in selected light- and medium-mass nuclei up to 56Ni. We derive an efficient scheme for including continuum effects in coupled-cluster computations of nuclei based on chiral nucleon-nucleon and three-nucleon forces, and present new results for unbound states in the neutron-rich isotopes of oxygen and calcium. The coupling to the continuum impacts the energies of the {J}π =1/{2}-,3/{2}-,7/{2}-,3/{2}+ states in {}{17,23,25}O, and—contrary to naive shell-model expectations—the level ordering of the {J}π =3/{2}+,5/{2}+,9/{2}+ states in {}{53,55,61}Ca. ).

  13. Limits on Lorentz Invariance Violation from Coulomb Interactions in Nuclei and Atoms.

    PubMed

    Flambaum, V V; Romalis, M V

    2017-04-07

    Anisotropy in the speed of light that has been constrained by Michelson-Morley-type experiments also generates anisotropy in the Coulomb interactions. This anisotropy can manifest itself as an energy anisotropy in nuclear and atomic experiments. Here the experimental limits on Lorentz violation in _{10}^{21}Ne are used to improve the limits on Lorentz symmetry violations in the photon sector, namely, the anisotropy of the speed of light and the Coulomb interactions, by 7 orders of magnitude in comparison with previous experiments: the speed of light is isotropic to a part in 10^{28}.

  14. Mass predictions from the Garvey-Kelson mass relations

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Jaenecke, J.; Masson, P.J.

    Part A: The transverse Garvey-Kelson mass relation represents a homogeneous third-order partial difference equation. Procedures are described for estimating masses of nuclei with Ngreater than or equal toZ from the most general solution of this difference equation subject to a chi/sup 2/ minimization, using the recent atomic mass adjustment of Wapstra, Audi, and Hoekstra as a boundary condition. A judicious division of the input data in subsets of neutron-rich and proton-rich nuclei had to be introduced to reduce systematic errors in long-range extrapolations. Approximately 5600 mass-excess values for nuclei with 2less than or equal toZless than or equal to103, 4lessmore » than or equal toNless than or equal to157, and Ngreater than or equal toZ (except N = Z odd for A<40) have been calculated. The standard deviation for reproducing the known mass-excess values is sigma/sub m/approx. =103 keV.« less

  15. The nuclear contacts and short range correlations in nuclei

    NASA Astrophysics Data System (ADS)

    Weiss, R.; Cruz-Torres, R.; Barnea, N.; Piasetzky, E.; Hen, O.

    2018-05-01

    Atomic nuclei are complex strongly interacting systems and their exact theoretical description is a long-standing challenge. An approximate description of nuclei can be achieved by separating its short and long range structure. This separation of scales stands at the heart of the nuclear shell model and effective field theories that describe the long-range structure of the nucleus using a mean-field approximation. We present here an effective description of the complementary short-range structure using contact terms and stylized two-body asymptotic wave functions. The possibility to extract the nuclear contacts from experimental data is presented. Regions in the two-body momentum distribution dominated by high-momentum, close-proximity, nucleon pairs are identified and compared to experimental data. The amount of short-range correlated (SRC) nucleon pairs is determined and compared to measurements. Non-combinatorial isospin symmetry for SRC pairs is identified. The obtained one-body momentum distributions indicate dominance of SRC pairs above the nuclear Fermi-momentum.

  16. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Winter, Frank; Detmold, William; Gambhir, Arjun S.

    The role of gluons in the structure of the nucleon and light nuclei is investigated using lattice quantum chromodynamics (QCD) calculations. The first moment of the unpolarised gluon distribution is studied in nuclei up to atomic numbermore » $A=3$ at quark masses corresponding to pion masses of $$m_\\pi\\sim 450$$ and $806$ MeV. Nuclear modification of this quantity defines a gluonic analogue of the EMC effect and is constrained to be less than $$\\sim 10$$% in these nuclei. This is consistent with expectations from phenomenological quark distributions and the momentum sum rule. In the deuteron, the combination of gluon distributions corresponding to the $$b_1$$ structure function is found to have a small first moment compared with the corresponding momentum fraction. The first moment of the gluon transversity structure function is also investigated in the spin-1 deuteron, where a non-zero signal is observed at $$m_\\pi \\sim 806$$ MeV. In conclusion, this is the first indication of gluon contributions to nuclear structure that can not be associated with an individual nucleon.« less

  17. The Z2/A dependence in heavy-ion fusion for the reactions of chlorine on thulium, lutetium, tantalum and tungsten. Final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    DiRienzo, A.C.

    1980-06-01

    Evaporation residues produced in the reactions 35Cl+169Tm and 37Cl+169Tm, 175Lu, 181Ta and 186W were observed at zero degree utilizing the Mass Inst of Tech.- Brookhaven Nat'l Lab Recoil Mass Spectrometer. The recoiling nuclei were separated from the beam and refocused onto a surface barrier detector by a combination of electrostatic and magnetic fields and magnetic quadrupole lenses. The residual nuclei are alpha radioactive and can thus be identified by a characteristic alpha line observed after the arrival pulse of the evaporation residue. The recoiling nuclei also pass through a gas ionization chamber whereas the decay alpha do not. A separatemore » anti-coincidence spectrum therefore displayed the alphas background free. Trends of evaporation residue cross section were charted versus Z sq (proton no.)/ A(atomic no.) and compared to statistical evaporation codes.« less

  18. Coulomb Excitation of Exotic Nuclei

    NASA Astrophysics Data System (ADS)

    Macchiavelli, Augusto O.

    2017-09-01

    The structure of nuclei far from the stability line is a central theme of research in nuclear physics. Key to this program has been the worldwide development of radioactive beam facilities and novel detector systems, which provide the tools needed to produce and study these exotic nuclei. Coulomb Excitation provides a unique probe to characterize the interplay of collective and single-particle degrees of freedom of the atomic nucleus. In particular, the combination of state-of-the-art charged particle detectors and gamma-ray spectroscopy plays a vital and ubiquitous role in these studies. As an introduction to this Mini-Symposium, I will present a short overview of this powerful technique and selected examples of recent experiments. Future opportunities with a 4 π gamma-ray tracking array like GRETA will be discussed. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Contract No. DE-AC02-05CH11231 (LBNL).

  19. Electron capture by U(91+) and U(92+) and ionization of U(90+) and U(91+)

    NASA Technical Reports Server (NTRS)

    Gould, H.; Greiner, D.; Lindstrom, P.; Symons, T. J. M.; Crawford, H.

    1984-01-01

    U(92+)/U(91+) and U(91+)/U(90+) electron-capture and ionization cross sections and equilibrium charge-state distributions are measured experimentally in mylar, Cu and Ta of varying thickness. Relativistic U(68+) ions at 437 or 962 MeV/nucleon are produced by a heavy-ion linear accelerator and synchrotron in tandem and passed through the target material into a magnetic specrometer and position-sensitive proportional counter for evaluation of charge states. The results are presented graphically and discussed. At 962 MeV/nucleon, beams containing 85 percent bare U(92+) nuclei are obtained using 150-mg/sq cm Cu or 85-mg/sq cm Ta; at 437 MeV/nucleon, 50 percent bare U(92+) nuclei are obtained with 90-mg/sq cm Cu. The techniques decribed can be applied to produce beams of bare U nuclei for acceleration to ultrarelativistic speeds or beams of few-electron U for atomic-physics experiments on quantum electrodynamics.

  20. SuperTIGER: On the Cosmic Ray Charge Frontier

    NASA Astrophysics Data System (ADS)

    Brandt, Theresa J.

    2017-08-01

    The Super Trans-Iron Galactic Element Recorder (SuperTIGER) was designed to measure significant statistics particularly for cosmic rays (CRs) with charge > 30. These heaviest nuclei are some 10^3-10^5 times rarer than the lighter elements. With the longest science flight to date on a Long Duration Balloon in 2012-13, SuperTIGER has collected >1200 of these rare nuclei and millions of lighter CR events. After the instrument spent two winters in Antarctica, we recovered it and are completing preparations for a second flight. We present results from the first flight, including the highest statistical precision measurements of CR charges from 30-40 to date. We anticipate even greater improvements with our second flight, this coming austral summer, 2017-18 from McMurdo, Antarctica. The results show enhanced numbers of elements formed in massive stars relative to solar system values, and thus give insight into the origin of Galactic CRs, likely in OB associations, and into the atomic processes which accelerate nuclei.

  1. Light Flashes Observed by Astronauts on Apollo 11 through Apollo 17.

    PubMed

    Pinsky, L S; Osborne, W Z; Bailey, J V; Benson, R E; Thompson, L F

    1974-03-08

    The crew members on the last seven Apollo flights observed light flashes that are tentatively attributed to cosmic ray nuclei (atomic number >/= 6) penetrating the head and eyes of the observers. Analyses of the event rates for all missions has revealed an anomalously low rate for transearth coast observations with respect to translunar coast observations.

  2. Maria Goeppert Mayer, the Nuclear Shell Structure, and Magic Numbers

    Science.gov Websites

    dropdown arrow Site Map A-Z Index Menu Synopsis Maria Goeppert-Mayer, the Nuclear Shell Model, and Magic explanation of how neutrons and protons within atomic nuclei are structured. Called the "nuclear shell American husband, chemical physicist Joseph Mayer. At Argonne, Goeppert-Mayer learned most of her nuclear

  3. Study of breakup and transfer of weakly bound nucleus 6Li to explore the low energy reaction dynamics

    NASA Astrophysics Data System (ADS)

    Zhang, G. L.; Zhang, G. X.; Hu, S. P.; Zhang, H. Q.; Gomes, P. R. S.; Lubian, J.; Guo, C. L.; Wu, X. G.; Yang, J. C.; Zheng, Y.; Li, C. B.; He, C. Y.; Zhong, J.; Li, G. S.; Yao, Y. J.; Guo, M. F.; Sun, H. B.; Valiente-Dobòn, J. J.; Goasduff, A.; Siciliano, M.; Galtarosa, F.; Francesco, R.; Testov, D.; Mengoni, D.; Bazzacco, D.; John, P. R.; Qu, W. W.; Wang, F.; Zheng, L.; Yu, L.; Chen, Q. M.; Luo, P. W.; Li, H. W.; Wu, Y. H.; Zhou, W. K.; Zhu, B. J.; Li, E. T.; Hao, X.

    2017-11-01

    Investigation of the breakup and transfer effect of weakly bound nuclei on the fusion process has been an interesting research topic in the past several years. However, owing to the low intensities of the presently available radioactive ion beam (RIB), it is difficult to clearly explore the reaction mechanisms of nuclear systems with unstable nuclei. In comparison with RIB, the beam intensities of stable weakly bound nuclei such as 6,7Li and 9Be, which have significant breakup probability, are orders of magnitude higher. Precise fusion measurements have already been performed with those stable weakly bound nuclei, and the effect of breakup of those nuclei on the fusion process has been extensively studied. Those nuclei indicated large production cross sections for particles other than the α + x breakup. The particles are originated from non-capture breakup (NCBU), incomplete fusion (ICF) and transfer processes. However, the conclusion of reaction dynamics was not clear and has the contradiction. In our previous experiments we have performed 6Li+96Zr and 154Sm at HI-13 Tandem accelerator of China Institute of Atomic Energy (CIAE) by using HPGe array. It is shown that there is a small complete fusion (CF) suppression on medium-mass target nucleus 96Zr different from about 35% suppression on heavier target nucleus 154Sm at near-barrier energies. It seems that the CF suppression factor depends on the charge of target nuclei. We also observed one neutron transfer process. However, the experimental data are scarce for medium-mass target nuclei. In order to have a proper understanding of the influence of breakup and transfer of weakly bound projectiles on the fusion process, we performed the 6Li+89Y experiment with incident energies of 22 MeV and 34 MeV on Galileo array in cooperation with Si-ball EUCLIDES at Legnaro National Laboratory (LNL) in Italy. Using particle-particle and particle-γ coincidences, the different reaction mechanisms can be clearly explored.

  4. Sub-barrier quasifission in heavy element formation reactions with deformed actinide target nuclei

    NASA Astrophysics Data System (ADS)

    Hinde, D. J.; Jeung, D. Y.; Prasad, E.; Wakhle, A.; Dasgupta, M.; Evers, M.; Luong, D. H.; du Rietz, R.; Simenel, C.; Simpson, E. C.; Williams, E.

    2018-02-01

    Background: The formation of superheavy elements (SHEs) by fusion of two massive nuclei is severely inhibited by the competing quasifission process. Low excitation energies favor SHE survival against fusion-fission competition. In "cold" fusion with spherical target nuclei near 208Pb, SHE yields are largest at beam energies significantly below the average capture barrier. In "hot" fusion with statically deformed actinide nuclei, this is not the case. Here the elongated deformation-aligned configurations in sub-barrier capture reactions inhibits fusion (formation of a compact compound nucleus), instead favoring rapid reseparation through quasifission. Purpose: To determine the probabilities of fast and slow quasifission in reactions with prolate statically deformed actinide nuclei, through measurement and quantitative analysis of the dependence of quasifission characteristics at beam energies spanning the average capture barrier energy. Methods: The Australian National University Heavy Ion Accelerator Facility and CUBE fission spectrometer have been used to measure fission and quasifission mass and angle distributions for reactions with projectiles from C to S, bombarding Th and U target nuclei. Results: Mass-asymmetric quasifission occurring on a fast time scale, associated with collisions with the tips of the prolate actinide nuclei, shows a rapid increase in probability with increasing projectile charge, the transition being centered around projectile atomic number ZP=14 . For mass-symmetric fission events, deviations of angular anisotropies from expectations for fusion fission, indicating a component of slower quasifission, suggest a similar transition, but centered around ZP˜8 . Conclusions: Collisions with the tips of statically deformed prolate actinide nuclei show evidence for two distinct quasifission processes of different time scales. Their probabilities both increase rapidly with the projectile charge. The probability of fusion can be severely suppressed by these two quasifission processes, since the sub-barrier heavy element yield is likely to be determined by the product of the probabilities of surviving each quasifission process.

  5. Shielding materials for highly penetrating space radiations

    NASA Technical Reports Server (NTRS)

    Kiefer, Richard L.; Orwoll, Robert A.

    1995-01-01

    Interplanetary travel involves the transfer from an Earth orbit to a solar orbit. Once outside the Earth's magnetosphere, the major sources of particulate radiation are solar cosmic rays (SCR's) and galactic cosmic rays (GCR's). Intense fluxes of SCR's come from solar flares and consist primarily of protons with energies up to 1 GeV. The GCR consists of a low flux of nuclei with energies up to 10(exp 10) GeV. About 70 percent of the GCR are protons, but a small amount (0.6 percent) are nuclei with atomic numbers greater than 10. High energy charged particles (HZE) interact with matter by transferring energy to atomic electrons in a Coulomb process and by reacting with an atomic nucleus. Energy transferred in the first process increases with the square of the atomic number, so particles with high atomic numbers would be expected to lose large amounts of energy by this process. Nuclear reactions produced by (HZE) particles produce high-energy secondary particles which in turn lose energy to the material. The HZE nuclei are a major concern for radiation protection of humans during interplanetary missions because of the very high specific ionization of both primary and secondary particles. Computer codes have been developed to calculate the deposition of energy by very energetic charged particles in various materials. Calculations show that there is a significant buildup of secondary particles from nuclear fragmentation and Coulomb dissociation processes. A large portion of these particles are neutrons. Since neutrons carry no charge, they only lose energy by collision or reaction with a nucleus. Neutrons with high energies transfer large amounts of energy by inelastic collisions with nuclei. However, as the neutron energy decreases, elastic collisions become much more effective for energy loss. The lighter the nucleus, the greater the fraction of the neutron's kinetic energy that can be lost in an elastic collision. Thus, hydrogen-containing materials such as polymers are most effective in reducing the energy of neutrons. Once neutrons are reduced to very low energies, the probability for undergoing a reaction with a nucleus (the cross section) becomes very high. The product of such a reaction is often radioactive and can involve the release of a significant amount of energy. Thus, it is important to provide protection from low energy neutrons during a long duration space flight. Among the light elements, lithium and boron each have an isotope with a large thermal neutron capture cross section, Li-6 and B-10. However, B-10 is more abundant in the naturally-occurring element than Li-6, has a thermal neutron capture cross section four times that of Li-6, and produces the stable products, He-4 and Li-7 in the interaction while Li-6 produces radioactive tritium (H-3). Thus, boron is the best light-weight material for thermal neutron absorption in spacecraft. The work on this project was focused in two areas: computer design where existing computer codes were used, and in some cases modified, to calculate the propagation and interactions of high energy charged particles through various media, and materials development where boron was incorporated into high performance materials.

  6. Atomic dynamics and the problem of the structural stability of free clusters of solidified inert gases

    NASA Astrophysics Data System (ADS)

    Verkhovtseva, É. T.; Gospodarev, I. A.; Grishaev, A. V.; Kovalenko, S. I.; Solnyshkin, D. D.; Syrkin, E. S.; Feodos'ev, S. B.

    2003-05-01

    The dependence of the rms amplitudes of atoms in free clusters of solidified inert gases on the cluster size is investigated theoretically and experimentally. Free clusters are produced by homogeneous nucleation in an adiabatically expanding supersonic stream. Electron diffraction is used to measure the rms amplitudes of the atoms; the Jacobi-matrix method is used for theoretical calculations. A series of distinguishing features of the atomic dynamics of microclusters was found. This was necessary to determine the character of the formation and the stability conditions of the crystal structure. It wass shown that for clusters consisting of less than N˜103 atoms, as the cluster size decreases, the rms amplitudes grow much more rapidly than expected from the increase in the specific contribution of the surface. It is also established that an fcc structure of a free cluster, as a rule, contains twinning defects (nuclei of an hcp phase). One reason for the appearance of such defects is the so-called vertex instability (anomalously large oscillation amplitudes) of the atoms in coordination spheres.

  7. Isomer depletion as experimental evidence of nuclear excitation by electron capture

    NASA Astrophysics Data System (ADS)

    Chiara, C. J.; Carroll, J. J.; Carpenter, M. P.; Greene, J. P.; Hartley, D. J.; Janssens, R. V. F.; Lane, G. J.; Marsh, J. C.; Matters, D. A.; Polasik, M.; Rzadkiewicz, J.; Seweryniak, D.; Zhu, S.; Bottoni, S.; Hayes, A. B.; Karamian, S. A.

    2018-02-01

    The atomic nucleus and its electrons are often thought of as independent systems that are held together in the atom by their mutual attraction. Their interaction, however, leads to other important effects, such as providing an additional decay mode for excited nuclear states, whereby the nucleus releases energy by ejecting an atomic electron instead of by emitting a γ-ray. This ‘internal conversion’ has been known for about a hundred years and can be used to study nuclei and their interaction with their electrons. In the inverse process—nuclear excitation by electron capture (NEEC)—a free electron is captured into an atomic vacancy and can excite the nucleus to a higher-energy state, provided that the kinetic energy of the free electron plus the magnitude of its binding energy once captured matches the nuclear energy difference between the two states. NEEC was predicted in 1976 and has not hitherto been observed. Here we report evidence of NEEC in molybdenum-93 and determine the probability and cross-section for the process in a beam-based experimental scenario. Our results provide a standard for the assessment of theoretical models relevant to NEEC, which predict cross-sections that span many orders of magnitude. The greatest practical effect of the NEEC process may be on the survival of nuclei in stellar environments, in which it could excite isomers (that is, long-lived nuclear states) to shorter-lived states. Such excitations may reduce the abundance of the isotope after its production. This is an example of ‘isomer depletion’, which has been investigated previously through other reactions, but is used here to obtain evidence for NEEC.

  8. Lorentz-like force emerging from kinematic interactions between electrons and nuclei in molecules: A quantum mechanical origin of symmetry breaking that can trigger molecular chirality.

    PubMed

    Takatsuka, Kazuo

    2017-02-28

    The Longuet-Higgins (Berry) phase arising from nonadiabatic dynamics and the Aharonov-Bohm phase associated with the dynamics of a charged particle in the electromagnetic vector potential are well known to be individually a manifestation of a class of the so-called geometrical phase. We herein discuss another similarity between the force working on a charged particle moving in a magnetic field, the Lorentz force, and a force working on nuclei while passing across a region where they have a strong quantum mechanical kinematic (nonadiabatic) coupling with electrons in a molecule. This kinematic force is indeed akin to the Lorentz force in that its magnitude is proportional to the velocity of the relevant nuclei and works in the direction perpendicular to its translational motion. Therefore this Lorentz-like nonadiabatic force is realized only in space of more or equal to three dimensions, thereby highlighting a truly multi-dimensional effect of nonadiabatic interaction. We investigate its physical significance qualitatively in the context of breaking of molecular spatial symmetry, which is not seen otherwise without this force. This particular symmetry breaking is demonstrated in application to a coplanar collision between a planar molecule and an atom sharing the same plane. We show that the atom is guided by this force to the direction out from the plane, resulting in a configuration that distinguishes one side of the mirror plane from the other. This can serve as a trigger for the dynamics towards molecular chirality.

  9. Direct Observation of Two Proton Radioactivity Using Digital Photography

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Rykaczewski, Krzysztof Piotr; Pfutzner, M.; Dominik, Wojciech

    2007-01-01

    Recently the observation of a new type of spontaneous radioactive decay has been claimed in which two protons are simultaneously ejected by an atomic nucleus from the ground state1,2,3. Experimental data obtained for the extremely neutron-deficient nuclei 45Fe and 54Zn, were interpreted as the first evidence of such a decay mode which has been sought since 1960.4 However, the technique applied in those studies allowed only measurements of the decay time and the total energy released. Particles emitted in the decay were not identified and the conclusions had to be supported by theoretical arguments. Here we show for the firstmore » time, directly and unambiguously, that 45Fe indeed disintegrates by two-proton decay. Furthermore, we demonstrate that the decay branch of this isotope leads to various particle emission channels including two-proton and three-proton emission. To achieve this result we have developed a new type of detector V the Optical Time Projection Chamber (OTPC) in which digital photography is applied to nuclear physics for the first time. The detector records images of tracks from charged particles, allowing for their unambiguous identification and the reconstruction of decay events in three dimensions. This new and simple technique provides a powerful method to identify exotic decay channels involving emission of charged particles. It is expected that further studies with the OTPC device will yield important information on nuclei located at and beyond the proton drip-line, thus providing new material for testing and improving models of very unstable atomic nuclei.« less

  10. Single-particle states vs. collective modes: friends or enemies ?

    NASA Astrophysics Data System (ADS)

    Otsuka, T.; Tsunoda, Y.; Togashi, T.; Shimizu, N.; Abe, T.

    2018-05-01

    The quantum self-organization is introduced as one of the major underlying mechanisms of the quantum many-body systems. In the case of atomic nuclei as an example, two types of the motion of nucleons, single-particle states and collective modes, dominate the structure of the nucleus. The collective mode arises as the balance between the effect of the mode-driving force (e.g., quadrupole force for the ellipsoidal deformation) and the resistance power against it. The single-particle energies are one of the sources to produce such resistance power: a coherent collective motion is more hindered by larger spacings between relevant single particle states. Thus, the single-particle state and the collective mode are "enemies" against each other. However, the nuclear forces are rich enough so as to enhance relevant collective mode by reducing the resistance power by changing single-particle energies for each eigenstate through monopole interactions. This will be verified with the concrete example taken from Zr isotopes. Thus, the quantum self-organization occurs: single-particle energies can be self-organized by (i) two quantum liquids, e.g., protons and neutrons, (ii) monopole interaction (to control resistance). In other words, atomic nuclei are not necessarily like simple rigid vases containing almost free nucleons, in contrast to the naïve Fermi liquid picture. Type II shell evolution is considered to be a simple visible case involving excitations across a (sub)magic gap. The quantum self-organization becomes more important in heavier nuclei where the number of active orbits and the number of active nucleons are larger.

  11. From J. J. Thomson to FAIR, what do we learn from Large-Scale Mass and Half-Life Measurements of Bare and Few-Electron Ions?

    NASA Astrophysics Data System (ADS)

    Münzenberg, Gottfried; Geissel, Hans; Litvinov, Yuri A.

    2010-04-01

    This contribution is based on the combination of the talks: "What can we learn from large-scale mass measurements," "Present and future experiments with stored exotic nuclei at relativistic energies," and "Beta decay of highly-charged ions." Studying the nuclear mass surface gives information on the evolution of nuclear structure such as nuclear shells, the onset of deformation and the drip-lines. Previously, most of the masses far-off stability has been obtained from decay data. Modern methods allow direct mass measurements. They are much more sensitive, down to single atoms, access short-lived species and have high accuracy. Large-scale explorations of the nuclear mass surface are ideally performed with the combination of the in-flight FRagment Separator FRS and the Experimental Storage Ring ESR. After a brief historic introduction selected examples such as the evolution of shell closures far-off stability and the proton-neutron interaction will be discussed in the framework of our data. Recently, the experiments have been extended and led to the discovery of new heavy neutron-rich isotopes along with their mass and lifetime measurements. Storage rings applied at relativistic energies are a unique tool to study the radioactive decay of bare or few-electron atomic nuclei. New features observed with the analysis of stored circulating mother and daughter ions including oscillations in the decay curves of hydrogen-like nuclei will be addressed. Future experiments with NUSTAR at FAIR will further extend our knowledge to the borderlines of nuclear existence.

  12. Measurement of the beta+ and orbital electron-capture decay rates in fully ionized, hydrogenlike, and heliumlike 140Pr ions.

    PubMed

    Litvinov, Yu A; Bosch, F; Geissel, H; Kurcewicz, J; Patyk, Z; Winckler, N; Batist, L; Beckert, K; Boutin, D; Brandau, C; Chen, L; Dimopoulou, C; Fabian, B; Faestermann, T; Fragner, A; Grigorenko, L; Haettner, E; Hess, S; Kienle, P; Knöbel, R; Kozhuharov, C; Litvinov, S A; Maier, L; Mazzocco, M; Montes, F; Münzenberg, G; Musumarra, A; Nociforo, C; Nolden, F; Pfützner, M; Plass, W R; Prochazka, A; Reda, R; Reuschl, R; Scheidenberger, C; Steck, M; Stöhlker, T; Torilov, S; Trassinelli, M; Sun, B; Weick, H; Winkler, M

    2007-12-31

    We report on the first measurement of the beta+ and orbital electron-capture decay rates of 140Pr nuclei with the simplest electron configurations: bare nuclei, hydrogenlike, and heliumlike ions. The measured electron-capture decay constant of hydrogenlike 140Pr58+ ions is about 50% larger than that of heliumlike 140Pr57+ ions. Moreover, 140Pr ions with one bound electron decay faster than neutral 140Pr0+ atoms with 59 electrons. To explain this peculiar observation one has to take into account the conservation of the total angular momentum, since only particular spin orientations of the nucleus and of the captured electron can contribute to the allowed decay.

  13. Detection prospects of the cosmic neutrino background

    NASA Astrophysics Data System (ADS)

    Li, Yu-Feng

    2015-04-01

    The existence of the cosmic neutrino background (CνB) is a fundamental prediction of the standard Big Bang cosmology. Although current cosmological probes provide indirect observational evidence, the direct detection of the CνB in a laboratory experiment is a great challenge to the present experimental techniques. We discuss the future prospects for the direct detection of the CνB, with the emphasis on the method of captures on beta-decaying nuclei and the PTOLEMY project. Other possibilities using the electron-capture (EC) decaying nuclei, the annihilation of extremely high-energy cosmic neutrinos (EHECνs) at the Z-resonance, and the atomic de-excitation method are also discussed in this review (talk given at the International Conference on Massive Neutrinos, Singapore, 9-13 February 2015).

  14. Measuring the Cosmic Particle Radiation from electrons to actinides - HNX/TIGERISS

    NASA Astrophysics Data System (ADS)

    Mitchell, John

    2017-01-01

    The Heavy Nuclei eXplorer (HNX) mission will measure the abundances of nuclei from Carbon (Z =6) to Curium (Z =96) in the cosmic radiation with the resolution to identify the atomic number of each detected nucleus. HNX will measure a significant number of actinides. HNX utilizes two high-precision instruments, the Extremely-heavy Cosmic-ray Composition Observer (ECCO) and the Cosmic-Ray Trans-Iron Galactic Element Recorder (CosmicTIGER), located in a SpaceX DragonLab capsule orbiting the Earth. This talk will discuss the motivating science, the HNX mission, the design and performance of the HNX instruments, and another new instrument, TIGERISS (Trans-Iron Galactic Element Recorder on the ISS), that will be proposed as an intermediate between SuperTIGER and HNX.

  15. Quantum Gas Microscope for Fermionic Atoms

    NASA Astrophysics Data System (ADS)

    Okan, Melih; Cheuk, Lawrence; Nichols, Matthew; Lawrence, Katherine; Zhang, Hao; Zwierlein, Martin

    2016-05-01

    Strongly interacting fermions define the properties of complex matter throughout nature, from atomic nuclei and modern solid state materials to neutron stars. Ultracold atomic Fermi gases have emerged as a pristine platform for the study of many-fermion systems. In this poster we demonstrate the realization of a quantum gas microscope for fermionic 40 K atoms trapped in an optical lattice and the recent experiments which allows one to probe strongly correlated fermions at the single atom level. We combine 3D Raman sideband cooling with high- resolution optics to simultaneously cool and image individual atoms with single lattice site resolution at a detection fidelity above 95%. The imaging process leaves the atoms predominantly in the 3D motional ground state of their respective lattice sites, inviting the implementation of a Maxwell's demon to assemble low-entropy many-body states. Single-site resolved imaging of fermions enables the direct observation of magnetic order, time resolved measurements of the spread of particle correlations, and the detection of many-fermion entanglement. NSF, AFOSR-PECASE, AFOSR-MURI on Exotic Phases of Matter, ARO-MURI on Atomtronics, ONR, a Grant from the Army Research Office with funding from the DARPA OLE program, and the David and Lucile Packard Foundation.

  16. A Nanotechnology Enhancement to Moore’s Law

    DTIC Science & Technology

    2013-01-01

    suggested that quantummechanics may be playing a role in consciousness , if a quantum mechanical model of mind and consciousness was developed, this would...necessary enhancement by an increasingly maturing nanotechnology and facing the inevitable quantum -mechanical atomic and nuclei limits. Since we cannot...important. (ii) Quantum computing: The other types of transistor material are rapidly developed in laboratories worldwide, for example, Spintronics

  17. Instrumentation for Applied Physics and Industrial Applications

    NASA Astrophysics Data System (ADS)

    Hillemanns, H.; Le Goff, J.-M.

    This document is part of Part 2 'Principles and Methods' of Subvolume B 'Detectors for Particles and Radiation' of Volume 21 'Elementary Particles' of Landolt-Börnstein - Group I 'Elementary Particles, Nuclei and Atoms'. It contains the Section '7.3 Instrumentation for Applied Physics and Industrial Applications' of Chapter '7 Applications of Detectors in Technology; Medicine and Other Fields' with the content:

  18. Three-Dimensional Nuclear Chart--Understanding Nuclear Physics and Nucleosynthesis in Stars

    ERIC Educational Resources Information Center

    Koura, Hiroyuki

    2014-01-01

    Three-dimensional (3D) nuclear charts were created using toy blocks, which represent the atomic masses per nucleon number and the total half-lives for each nucleus in the entire region of the nuclear mass. The bulk properties of the nuclei can be easily understood by using these charts. Subsequently, these charts were used in outreach activities…

  19. The quantum universe

    NASA Astrophysics Data System (ADS)

    Hey, Anthony J. G.; Walters, Patrick

    This book provides a descriptive, popular account of quantum physics. The basic topics addressed include: waves and particles, the Heisenberg uncertainty principle, the Schroedinger equation and matter waves, atoms and nuclei, quantum tunneling, the Pauli exclusion principle and the elements, quantum cooperation and superfluids, Feynman rules, weak photons, quarks, and gluons. The applications of quantum physics to astrophyics, nuclear technology, and modern electronics are addressed.

  20. Approximate symmetries in atomic nuclei from a large-scale shell-model perspective

    NASA Astrophysics Data System (ADS)

    Launey, K. D.; Draayer, J. P.; Dytrych, T.; Sun, G.-H.; Dong, S.-H.

    2015-05-01

    In this paper, we review recent developments that aim to achieve further understanding of the structure of atomic nuclei, by capitalizing on exact symmetries as well as approximate symmetries found to dominate low-lying nuclear states. The findings confirm the essential role played by the Sp(3, ℝ) symplectic symmetry to inform the interaction and the relevant model spaces in nuclear modeling. The significance of the Sp(3, ℝ) symmetry for a description of a quantum system of strongly interacting particles naturally emerges from the physical relevance of its generators, which directly relate to particle momentum and position coordinates, and represent important observables, such as, the many-particle kinetic energy, the monopole operator, the quadrupole moment and the angular momentum. We show that it is imperative that shell-model spaces be expanded well beyond the current limits to accommodate particle excitations that appear critical to enhanced collectivity in heavier systems and to highly-deformed spatial structures, exemplified by the second 0+ state in 12C (the challenging Hoyle state) and 8Be. While such states are presently inaccessible by large-scale no-core shell models, symmetry-based considerations are found to be essential.

  1. High-precision evaluation of the magnetic moment of the helion

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Neronov, Yu. I., E-mail: yineronov@mail.ru; Seregin, N. N.

    NMR spectra of samples containing a mixture of hydrogen deuteride HD with pressure of about 80 atm and helium-3 with partial pressure of about 1 atm are analyzed. The ratio of the resonance frequencies of the nuclei, F({sup 3}He)/F(H{sub 2}), is determined to be 0.761786594(2), which is equal to the magnetic moment of the helion (bound in a helium atom) in the units of the magnetic moment of a proton (bound in molecular hydrogen). The uncertainty of two digits in the last place corresponds to a relative error of {delta}[F({sup 3}He)/F(H{sub 2})] = 2.6 Multiplication-Sign 10{sup -9}. The use ofmore » the known calculated data on the shielding of nuclei in the helium-3 atom ({sigma}({sup 3}He) = 59924(2) Multiplication-Sign 10{sup -9}) and on the shielding of protons in hydrogen ({sigma}(H{sub 2}) = 26288(2) Multiplication-Sign 10{sup -9}) yields a value of {mu}({sup 3}He)/{mu}{sub p} = -0.761812217(3) for the free magnetic moment of the helion in the units of the proton magnetic moment.« less

  2. Proton-proton correlations observed in two-proton radioactivity of 94Ag.

    PubMed

    Mukha, Ivan; Roeckl, Ernst; Batist, Leonid; Blazhev, Andrey; Döring, Joachim; Grawe, Hubert; Grigorenko, Leonid; Huyse, Mark; Janas, Zenon; Kirchner, Reinhard; La Commara, Marco; Mazzocchi, Chiara; Tabor, Sam L; Van Duppen, Piet

    2006-01-19

    The stability and spontaneous decay of naturally occurring atomic nuclei have been much studied ever since Becquerel discovered natural radioactivity in 1896. In 1960, proton-rich nuclei with an odd or an even atomic number Z were predicted to decay through one- and two-proton radioactivity, respectively. The experimental observation of one-proton radioactivity was first reported in 1982, and two-proton radioactivity has now also been detected by experimentally studying the decay properties of 45Fe (refs 3, 4) and 54Zn (ref. 5). Here we report proton-proton correlations observed during the radioactive decay of a spinning long-lived state of the lightest known isotope of silver, 94Ag, which is known to undergo one-proton decay. We infer from these correlations that the long-lived state must also decay through simultaneous two-proton emission, making 94Ag the first nucleus to exhibit one- as well as two-proton radioactivity. We attribute the two-proton emission behaviour and the unexpectedly large probability for this decay mechanism to a very large deformation of the parent nucleus into a prolate (cigar-like) shape, which facilitates emission of protons either from the same or from opposite ends of the 'cigar'.

  3. Emergent properties of nuclei from ab initio coupled-cluster calculations

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hagen, G.; Hjorth-Jensen, M.; Jansen, G. R.

    Emergent properties such as nuclear saturation and deformation, and the effects on shell structure due to the proximity of the scattering continuum and particle decay channels are fascinating phenomena in atomic nuclei. In recent years, ab initio approaches to nuclei have taken the first steps towards tackling the computational challenge of describing these phenomena from Hamiltonians with microscopic degrees of freedom. Our endeavor is now possible due to ideas from effective field theories, novel optimization strategies for nuclear interactions, ab initio methods exhibiting a soft scaling with mass number, and ever-increasing computational power. We review some of the recent accomplishments. We also present new results. The recently optimized chiral interaction NNLOmore » $${}_{{\\rm{sat}}}$$ is shown to provide an accurate description of both charge radii and binding energies in selected light- and medium-mass nuclei up to 56Ni. We derive an efficient scheme for including continuum effects in coupled-cluster computations of nuclei based on chiral nucleon–nucleon and three-nucleon forces, and present new results for unbound states in the neutron-rich isotopes of oxygen and calcium. Finally, the coupling to the continuum impacts the energies of the $${J}^{\\pi }=1/{2}^{-},3/{2}^{-},7/{2}^{-},3/{2}^{+}$$ states in $${}^{\\mathrm{17,23,25}}$$O, and—contrary to naive shell-model expectations—the level ordering of the $${J}^{\\pi }=3/{2}^{+},5/{2}^{+},9/{2}^{+}$$ states in $${}^{\\mathrm{53,55,61}}$$Ca.« less

  4. Emergent properties of nuclei from ab initio coupled-cluster calculations

    DOE PAGES

    Hagen, G.; Hjorth-Jensen, M.; Jansen, G. R.; ...

    2016-05-17

    Emergent properties such as nuclear saturation and deformation, and the effects on shell structure due to the proximity of the scattering continuum and particle decay channels are fascinating phenomena in atomic nuclei. In recent years, ab initio approaches to nuclei have taken the first steps towards tackling the computational challenge of describing these phenomena from Hamiltonians with microscopic degrees of freedom. Our endeavor is now possible due to ideas from effective field theories, novel optimization strategies for nuclear interactions, ab initio methods exhibiting a soft scaling with mass number, and ever-increasing computational power. We review some of the recent accomplishments. We also present new results. The recently optimized chiral interaction NNLOmore » $${}_{{\\rm{sat}}}$$ is shown to provide an accurate description of both charge radii and binding energies in selected light- and medium-mass nuclei up to 56Ni. We derive an efficient scheme for including continuum effects in coupled-cluster computations of nuclei based on chiral nucleon–nucleon and three-nucleon forces, and present new results for unbound states in the neutron-rich isotopes of oxygen and calcium. Finally, the coupling to the continuum impacts the energies of the $${J}^{\\pi }=1/{2}^{-},3/{2}^{-},7/{2}^{-},3/{2}^{+}$$ states in $${}^{\\mathrm{17,23,25}}$$O, and—contrary to naive shell-model expectations—the level ordering of the $${J}^{\\pi }=3/{2}^{+},5/{2}^{+},9/{2}^{+}$$ states in $${}^{\\mathrm{53,55,61}}$$Ca.« less

  5. Heavy Metal Stars

    NASA Astrophysics Data System (ADS)

    2001-08-01

    La Silla Telescope Detects Lots of Lead in Three Distant Binaries Summary Very high abundances of the heavy element Lead have been discovered in three distant stars in the Milky Way Galaxy . This finding strongly supports the long-held view that roughly half of the stable elements heavier than Iron are produced in common stars during a phase towards the end of their life when they burn their Helium - the other half results from supernova explosions. All the Lead contained in each of the three stars weighs about as much as our Moon. The observations show that these "Lead stars" - all members of binary stellar systems - have been more enriched with Lead than with any other chemical element heavier than Iron. This new result is in excellent agreement with predictions by current stellar models about the build-up of heavy elements in stellar interiors. The new observations are reported by a team of Belgian and French astronomers [1] who used the Coude Echelle Spectrometer on the ESO 3.6-m telescope at the La Silla Observatory (Chile). PR Photo 26a/01 : A photo of HD 196944 , one of the "Lead stars". PR Photo 26b/01 : A CES spectrum of HD 196944 . The build-up of heavy elements Astronomers and physicists denote the build-up of heavier elements from lighter ones as " nucleosynthesis ". Only the very lightest elements (Hydrogen, Helium and Lithium [2]) were created at the time of the Big Bang and therefore present in the early universe. All the other heavier elements we now see around us were produced at a later time by nucleosynthesis inside stars. In those "element factories", nuclei of the lighter elements are smashed together whereby they become the nuclei of heavier ones - this process is known as nuclear fusion . In our Sun and similar stars, Hydrogen is being fused into Helium. At some stage, Helium is fused into Carbon, then Oxygen, etc. The fusion process requires positively charged nuclei to move very close to each other before they can unite. But with increasing atomic mass and hence, increasing positive charge of the nuclei, the electric repulsion between the nuclei becomes stronger and stronger. In fact, the fusion process only works up to a certain mass limit, corresponding to the element Iron [2]. All elements that are heavier than Iron cannot be produced via this path. But then, how were those heavy elements we now find on the Earth produced in the first place? From where comes the Zirconium in artificial diamonds, the Barium that colours fireworks, the Tungsten in the filaments in electric bulbs? Which process made the Lead in your car battery? Beyond iron The production of elements heavier than Iron takes place by adding neutrons to the atomic nuclei . These neutral particles do not feel any electrical repulsion from the charged nuclei. They can therefore easily approach them and thereby create heavier nuclei. This is indeed the way the heaviest chemical elements are built up. There are actually two different stellar environments where this process of "neutron capture" can happen. One place where this process occurs is inside very massive stars when they explode as supernovae . In such a dramatic event, the build-up proceeds very rapidly, via the so-called "r-process" ( "r" for rapid ). The AGB stars But not all heavy elements are created in such an explosive way. A second possibility follows a more "peaceful" road. It takes place in rather normal stars, when they burn their Helium towards the end of their lives. In the so-called "s-process" ( "s" for slow ), heavier elements are then produced by a rather gentle addition of neutral neutrons to atomic nuclei. In fact, roughly half of all the elements heavier than Iron are believed to be synthesized by this process during the late evolutionary phases of stars. This process takes place during a specific stage of stellar evolution, known as the "AGB" phase [3]. It occurs just before an old star expels its gaseous envelope into the surrounding interstellar space and sometime thereafter dies as a burnt-out, dim "white dwarf" . Stars with masses between 0.8 and 8 times that of the Sun are believed to evolve to AGB-stars and to end their lives in this particular way. At the same time, they produce beautiful nebulae like the "Dumbbell Nebula". Our Sun will also end its active life this way, probably some 7 billion years from now. Low-metallicity stars The detailed understanding of the "s-process" and, in particular, where it takes place inside an AGB-star, has been an area of active research for many years. Current state-of-the-art computer-based stellar models predict that the s-process should be particularly efficient in stars with a comparatively low content of metals ("metal-poor" or "low-metallicity" stars) . In such stars - which were born at an early epoch in our Galaxy and are therefore quite old - the "s-process" is expected to effectively produce atomic nuclei all the way up to the most heavy, stable ones, like Lead (atomic number 82 [2]) and Bismuth (atomic number 83) - since more neutrons are available per Iron-seed nucleus when there are fewer such nuclei (as compared to the solar composition). Once these elements have been produced, the addition of more s-process neutrons to those nuclei will only produce unstable elements that decay back to Lead. Hence, when the s-process is sufficiently efficient, atomic nuclei with atomic numbers around 82, that is, the Lead region, just continue to pile up. As a result, when compared to stars with "normal" abundances of the metals (like our Sun), those low-metallicity stars should thus exhibit a significant "over-abundance" of those very heavy elements with respect to Iron, in particular of Lead . Looking for Lead Direct observational support for this theoretical prediction would be the discovery of some low-metallicity stars with a high abundance of Lead. At the same time, the measured amounts of all the heavy elements and their relative abundances would provide very valuable information and strongly reinforce our current understanding of heavy element nucleosynthesis. But detecting the element Lead is not easy - the expected spectral lines of Lead in stellar spectra are relatively weak, and they are blended with many nearby absorption lines of other elements. Moreover, bona-fide, low-metallicity AGB stars appear to be extremely rare in the solar neighborhood . But if the necessary observations are so difficult, how is it then possible to probe nucleosynthesis in low-metallicity AGB stars? CH-stars in binary systems ESO PR Photo 26a/01 ESO PR Photo 26a/01 [Preview - JPEG: 350 x 400 pix - 232k] [Normal - JPEG: 700 x 800 pix - 616k] Caption : One of the three Lead stars, HD 196944 that was analyzed in the present research programme (at the center of the field). This star lies about 1600 light years away in the constellation Aquarius. At magnitude 9, it is not visible to the unaided eye, but easily seen through a small amateur telescope. Still, the detailed spectroscopic study reported in this Press release that revealed a high abundance of Lead in this star required a 4-m class telescope. This DSS-image are copyright by the UK SERC/PPARC (Particle Physics and Astronomy Research Council, formerly Science and Engineering Research Council), the Anglo-Australian Telescope Board and the Association of Universities for Research in Astronomy (AURA). The spikes seen in this photo are an optical effect in the telescope. In a determined effort in this direction, a team of Belgian and French astronomers [1] decided to try to detect the presence of Lead in some "CH-stars" [4] that are located about 1600 light-years away, high above the main plane of our Milky Way Galaxy. Over-abundance of some heavy elements has been observed in some "CH-stars". But CH-stars are not very luminous and have not yet evolved to the AGB phase. Hence they are totally unable to produce heavy elements. So how can there be heavy elements in the CH-stars? This mystery was solved when it was realized that the CH-stars all belong to binary systems and that they therefore have a companion star [5]. That companion is now a white dwarf star and was therefore at some earlier moment an AGB star ! During its AGB-phase, the companion star expelled much of its material, eventually producing the "planetary nebula" phenomenon, referred to above. In this process, a lot of its material, enriched with heavy elements produced by the "s-process" during the AGB phase, was deposited in the atmosphere of the CH-star that is now observed. The former AGB-star, now a slowly cooling, dim white-dwarf star, still orbits the CH-star. For this reason, the atmospheric composition of a CH-star actually carries the signature of the nucleosynthesis that took place deep inside the companion AGB star at an earlier epoch. Spectroscopic observations of CH-stars thus provide the opportunity to probe the predicted s-process in low-metallicity stars. Three stars with Lead ESO PR Photo 26b/01 ESO PR Photo 26b/01 [Preview - JPEG: 400 x 371 pix - 95k] [Normal - JPEG: 800 x 741 pix - 240k] Caption : A high-resolution spectrum of the CH-star HD 196944, obtained with the CES instrument on the ESO 3.6-m telescope in September 2000. The observed spectrum (dots) shows many absorption lines from elements that are usually seen in stars. The red line shows a model in which elements (in particular those produced by the s-process) are present in normal quantities, compared to Iron. The blue line instead shows a model where s-processing has occured. It is obvious that the red line does not fit, only the blue line reproduces the observed absorption line at wavelength 405.781 nm caused by Lead (Pb) atoms in the atmosphere of this star. A subsequent, detailed analysis demonstrated that HD 196944 is a true "Lead star". Technical information about this photo is available below. A necessary condition for these observations to succeed is a very high spectral resolution in order to detect the spectral line of Lead (Pb), in particular to "resolve" it among the many absorption lines from other elements, present in the stellar spectrum in this wavelength region. Moreover, a fairly large telescope is needed as the stars to be observed are relatively rare, hence distant and faint for this kind of demanding observations. The Belgian and French astronomers decided to use the Coude Echelle Spectrometer (CES) at the ESO 3.6-m telescope on La Silla, a telescope/instrument combination offering some hope of success for these difficult observations. Spectra of three southern stars, HD 187861, HD 196944 and HD 224959 , were obtained during two nights in September 2000 and found to be of excellent quality. The scientists were very pleased to find that the Lead absorption line was clearly present and very strong in the spectra of all three stars . A subsequent, detailed analysis demonstrated that the three stars all have a substantial overabundance of Lead. Moreover, from the measured abundances of other elements in these spectra, it is also clear that this Lead has been formed in the s-process . The astronomers were able to prove that the Lead cannot originate from the competing "r-process" that occurs in other environments like supernova explosions. " This is the first detection of a Lead-star ", explains Sophie Van Eck from the Institut d'Astronomie et d'Astrophysique of the Université Libre de Bruxelles (Belgium). " These stars are almost exclusively enriched with Lead. Moreover, the abundances in all three stars show a remarkable similarity ." How does the s-process operate? The high abundance of Lead in these otherwise low-metallicity stars also provides detailed clues on how the s-process operates inside the AGB stars. When a Carbon-13 nucleus (i.e. a nucleus with 6 protons and 7 neutrons [2]) is hit by a Helium-4 nucleus (2 protons and 2 neutrons), they fuse to form Oxygen-16 (8 protons and 8 neutrons). In this process - as can be seen by adding the numbers - one neutron is released. It is exactly these surplus neutrons that become the building-blocks for making heavier elements via the s-process. Hence the true source of the required neutrons is the Carbon-13 isotope, which is in turn produced by fusion of normal carbon (Carbon-12) and protons, i.e. hydrogen nuclei. However, an additional problem is that it seems that nowhere inside the star would there be sufficient Carbon and Hydrogen in the same place to allow this process to take off. Indeed most hydrogen nuclei have already been "used up" and have fused to heavier nuclei, including Carbon. But the observations now prove that the s-process does happen - how is this then possible? Mixing the star Current models of stellar interiors suggest that a moderate, "partial" mixing occurs that occasionally drags Hydrogen down to the Carbon-rich inner regions (and some Carbon moves up into the Hydrogen-rich region). It is still not clearly understood exactly how this process operates, but the Belgian astronomers independently predicted that if such a "partial mixing process" does take place in a low-metallicity star, then Lead-stars should exist and it should also be possible to observe them. " Our discovery of these Lead stars is without any doubt the clearest signature of that model prediction we have today ", states Sophie Van Eck . " The excellent agreement between predicted and observed abundances reinforces our current understanding of the detailed operation of the s-process in the deep interiors of the stars, and thus constitutes an important piece of information on how the heaviest stable elements in the universe are formed ." Three moons and your car battery The astronomers altogether found a mass of Lead in each of the three stars that is about the same as the mass of our Moon (7.4 x 10 22 kg). Stars like these were once the most efficient Lead factories in the Universe. It is likely that the Lead in your car battery was once produced in such a low-metallicity star. From that star, it was later dispersed into the interstellar medium and was present in the cloud of dust and gas from which the Solar System and hence our Earth was formed. More information The research described in this Press Release is reported in a scientific article ("Discovery of three Lead stars" by S. Van Eck, S. Goriely, A. Jorissen and B. Plez) that appears in the August 23, 2001 issue of the science journal "Nature". Notes [1]: The team consists of Sophie Van Eck , Stéphane Goriely , Alain Jorissen (all Institut d'Astronomie et d'Astrophysique de l'Université Libre de Bruxelles, Belgium) and Bertrand Plez (Groupe de Recherche en Astronomie et Astrophysique en Languedoc, Université de Montpellier II - GRAAL), France). Sophie Van Eck was an ESO fellow (1999-2000). [2] The "atomic mass" of a chemical element is the total mass of the positively charged protons and neutral neutrons in the atomic nucleus. The "atomic number" of a chemical element is equal to the number of protons in the nucleus. Different isotopes of a chemical element all have the same number of protons in the nuclei, but a different number of neutrons. For the principal (most abundant) isotopes of the elements mentioned in this text, the "atomic mass" (expressed in "atomic mass units" (amu)) is approximately: Hydrogen : 1 atomic mass unit (with 1 proton in the nucleus); Helium : 4 atomic mass units (2 protons + 2 neutrons); Lithium : 7 atomic mass units (3 protons + 4 neutrons); Carbon : 12 atomic mass units (6 protons + 6 neutrons); Oxygen : 16 atomic mass units (8 protons + 8 neutrons); Iron : 56 atomic mass units (26 protons + 30 neutrons); Zirconium : 90 atomic mass units (40 protons + 50 neutrons); Barium : 138 atomic mass units (56 protons + 82 neutrons); Tungsten : 184 atomic mass units (74 protons + 110 neutrons); Lead : 208 atomic mass units (82 protons + 126 neutrons); Bismuth : 209 atomic mass units (83 protons + 126 neutrons) [3] "AGB" stands for "Asymptotic Giant Branch"; a location in the HR-diagramme (a plot of stellar colours and luminosities) of evolved stars in which hydrogen and helium burning occurs in two concentric shells and elements heavier than iron are produced via the s-process. [4] The "CH-stars" owe their name to the prominent bands of the CH-molecule observed in their spectrum. [5] The fact that CH-stars are all double stars was discovered by the Canadian astronomer Robert McClure in 1984. Technical information about the photos PR Photo 26b/01 shows a small section of the reduced spectrum of the CH-star HD 196944, near wavelength 4050 Angstrom. It was obtained during a 90-min exposure with the Coude Echelle Spectrometer at the ESO 3.6-m telescope on La Silla in 16 September 2000. The spectral resolution is 135 000.

  6. Global and local approaches to population analysis: Bonding patterns in superheavy element compounds

    NASA Astrophysics Data System (ADS)

    Oleynichenko, Alexander; Zaitsevskii, Andréi; Romanov, Stepan; Skripnikov, Leonid V.; Titov, Anatoly V.

    2018-03-01

    Relativistic effective atomic configurations of superheavy elements Cn, Nh and Fl and their lighter homologues (Hg, Tl and Pb) in their simple compounds with fluorine and oxygen are determined using the analysis of local properties of molecular Kohn-Sham density matrices in the vicinity of heavy nuclei. The difference in populations of atomic spinors with the same orbital angular momentum and different total angular momenta is demonstrated to be essential for understanding the peculiarities of chemical bonding in superheavy element compounds. The results are fully compatible with those obtained by the relativistic iterative version of conventional projection analysis of global density matrices.

  7. Masses and β -Decay Spectroscopy of Neutron-Rich Odd-Odd Eu,162160 Nuclei: Evidence for a Subshell Gap with Large Deformation at N =98

    NASA Astrophysics Data System (ADS)

    Hartley, D. J.; Kondev, F. G.; Orford, R.; Clark, J. A.; Savard, G.; Ayangeakaa, A. D.; Bottoni, S.; Buchinger, F.; Burkey, M. T.; Carpenter, M. P.; Copp, P.; Gorelov, D. A.; Hicks, K.; Hoffman, C. R.; Hu, C.; Janssens, R. V. F.; Klimes, J. W.; Lauritsen, T.; Sethi, J.; Seweryniak, D.; Sharma, K. S.; Zhang, H.; Zhu, S.; Zhu, Y.

    2018-05-01

    The structure of deformed neutron-rich nuclei in the rare-earth region is of significant interest for both the astrophysics and nuclear structure fields. At present, a complete explanation for the observed peak in the elemental abundances at A ˜160 eludes astrophysicists, and models depend on accurate quantities, such as masses, lifetimes, and branching ratios of deformed neutron-rich nuclei in this region. Unusual nuclear structure effects are also observed, such as the unexpectedly low energies of the first 2+ levels in some even-even nuclei at N =98 . In order to address these issues, mass and β -decay spectroscopy measurements of the Eu97 160 and Eu99 162 nuclei were performed at the Californium Rare Isotope Breeder Upgrade radioactive beam facility at Argonne National Laboratory. Evidence for a gap in the single-particle neutron energies at N =98 and for large deformation (β2˜0.3 ) is discussed in relation to the unusual phenomena observed at this neutron number.

  8. Observing electron localization in a dissociating H2+ molecule in real time

    PubMed Central

    Xu, H.; Li, Zhichao; He, Feng; Wang, X.; Atia-Tul-Noor, A.; Kielpinski, D.; Sang, R. T.; Litvinyuk, I. V.

    2017-01-01

    Dissociation of diatomic molecules with odd number of electrons always causes the unpaired electron to localize on one of the two resulting atomic fragments. In the simplest diatomic molecule H2+ dissociation yields a hydrogen atom and a proton with the sole electron ending up on one of the two nuclei. That is equivalent to breaking of a chemical bond—the most fundamental chemical process. Here we observe such electron localization in real time by performing a pump–probe experiment. We demonstrate that in H2+ electron localization is complete in just 15 fs when the molecule’s internuclear distance reaches 8 atomic units. The measurement is supported by a theoretical simulation based on numerical solution of the time-dependent Schrödinger equation. This observation advances our understanding of detailed dynamics of molecular dissociation. PMID:28621332

  9. The quest for novel modes of excitation in exotic nuclei

    NASA Astrophysics Data System (ADS)

    Paar, N.

    2010-06-01

    This paper provides an insight into several open problems in the quest for novel modes of excitation in nuclei with isospin asymmetry, deformation and finite-temperature characteristics in stellar environments. Major unsolved problems include the nature of pygmy dipole resonances, the quest for various multipole and spin-isospin excitations both in neutron-rich and proton drip-line nuclei mainly driven by loosely bound nucleons, excitations in unstable deformed nuclei and evolution of their properties with the shape phase transition. Exotic modes of excitation in nuclei at finite temperatures characteristic of supernova evolution present open problems with a possible impact in modeling astrophysically relevant weak interaction rates. All these issues challenge self-consistent many-body theory frameworks at the frontiers of on-going research, including nuclear energy density functionals, both phenomenological and constrained by the strong interaction physics of QCD, models based on low-momentum two-nucleon interaction Vlow-k and correlated realistic nucleon-nucleon interaction VUCOM, supplemented by three-body force, as well as two-nucleon and three-nucleon interactions derived from the chiral effective field theory. Joined theoretical and experimental efforts, including research with radioactive isotope beams, are needed to provide insight into dynamical properties of nuclei away from the valley of stability, involving the interplay of isospin asymmetry, deformation and finite temperature.

  10. FROM THE HISTORY OF PHYSICS: The development of the first Soviet atomic bomb

    NASA Astrophysics Data System (ADS)

    Goncharov, German A.; Ryabev, Lev D.

    2001-01-01

    In the late 1930s and early 1940s, two remarkable physical phenomena — the fission of heavy nuclei and the chain fission reaction — were discovered, implying that a new powerful source of energy (nuclear fission energy) might become a practical possibility for mankind. At that time, however, the political situation in the world made the development of the atomic bomb the main objective of nuclear energy research in the countries involved. The first atomic bombs, notoriously used in the war against Japan, were produced by the United States of America only six and a half years after the discovery of fission. Four years later, the first Soviet atomic bomb was tested. This was a major step toward the establishment of nuclear parity which led to stability and global peace and thus greatly influenced the destiny of human kind. Based on documentary materials covering the period from 1939 to 1949, this paper traces the origin and evolution of the physical ideas behind the first Soviet atomic bomb and discusses the most important events associated with the project.

  11. Superheavy-element spectroscopy: Correlations along element 115 decay chains

    NASA Astrophysics Data System (ADS)

    Rudolph, D.; Forsberg, U.; Sarmiento, L. G.; Golubev, P.; Fahlander, C.

    2016-05-01

    Following a brief summary of the region of the heaviest atomic nuclei yet created in the laboratory, data on more than hundred α-decay chains associated with the production of element 115 are combined to investigate time and energy correlations along the observed decay chains. Several of these are analysed using a new method for statistical assessments of lifetimes in sets of decay chains.

  12. Nuclear Physics Around the Unitarity Limit.

    PubMed

    König, Sebastian; Grießhammer, Harald W; Hammer, H-W; van Kolck, U

    2017-05-19

    We argue that many features of the structure of nuclei emerge from a strictly perturbative expansion around the unitarity limit, where the two-nucleon S waves have bound states at zero energy. In this limit, the gross features of states in the nuclear chart are correlated to only one dimensionful parameter, which is related to the breaking of scale invariance to a discrete scaling symmetry and set by the triton binding energy. Observables are moved to their physical values by small perturbative corrections, much like in descriptions of the fine structure of atomic spectra. We provide evidence in favor of the conjecture that light, and possibly heavier, nuclei are bound weakly enough to be insensitive to the details of the interactions but strongly enough to be insensitive to the exact size of the two-nucleon system.

  13. Nuclear Data Evaluation for Mass Chain A=217:Odd-Proton Nuclei

    PubMed Central

    Nafee, Sherif S.; Shaheen, Salem A.; Al-Ramady, Amir M.

    2016-01-01

    Thallium (Tl81217), Bismuth (Bi83217), Astatine (At85217), Francium (Fr87217), Actinium (Ac89217) and Protactinium (Pa91217) are of odd-proton numbers among the mass chain A = 217. In the present work, the half-lives and gamma transitions for the six nuclei have been studied and adopted based on the recently published interactions or unevaluated nuclear data sets XUNDL. The Q (α) has been updated based on the recent published work of the Atomic Mass Evaluation AME2012 as well. Moreover, the total conversion electrons as well as the K-Shell to L-Shell, L-Shell to M-Shell and L-Shell to N-Shell Conversion Electron Ratios have been calculated using BrIcc code v2.3. An updated skeleton decay scheme for each of the above nuclei has been presented here. The decay hindrance factors (HF) calculated using the ALPHAD program, which is available from Brookhaven National Laboratory’s website, have been calculated for the α- decay data sets for 221Fr-, 221Ac- and 221Pa- α-decays. PMID:26761207

  14. Rare isotopes and the sound of dilute nuclear matter

    NASA Astrophysics Data System (ADS)

    Papakonstantinou, P.

    2018-04-01

    Dilute baryonic matter, at densities below the normal saturation density of symmetric matter, is found on the crust of neutron stars and in collapsing supernova matter, its properties determining the evolution of those stellar objects. It is also readily found on the surface of ordinary and exotic atomic nuclei and lives fleetingly in the form of space-extended resonances of excited nucleons. Liminal states of nuclear matter, between saturation and full evaporation or clusterization, are manifest in the structure of symmetric nuclei through clustering and of very asymmetric rare species in haloes and the neutron skin; they stand literally at the threshold of a nucleus's response to hadronic probes, including processes which hinder or enable fusion. In this contribution I focus on excited states, and in particular exotic or not-so-exotic dipole excitation modes of N = Z nuclei and neutron-rich species, including new theoretical results on threshold strength. Modes of special interest are vibrations of and within diffuse surface layers and alpha-cluster oscillations. The modeling of such processes is relevant, directly or indirectly, for the description of reactions at astrophysical energies.

  15. Infrared coronal emission lines and the possibility of their laser emission in Seyfert nuclei

    NASA Technical Reports Server (NTRS)

    Greenhouse, Matthew A.; Feldman, Uri; Smith, Howard A.; Klapisch, Marcel; Bhatia, Anand K.; Bar-Shalom, Avi

    1993-01-01

    Results are presented from detailed balance calculations, and a compilation of atomic data and other model calculations designed to support upcoming ISO and current observing programs involving IR coronal emission lines, together with a table with a complete line list of infrared transitions within the ground configurations 2s2 2p(k), 3s2 3p(k), and the first excited configurations 2s 2p and 3s 3p of highly ionized astrophysically abundant elements. The temperature and density parameter space for dominant cooling via IR coronal lines is presented, and the relationship of IR and optical coronal lines is discussed. It is found that, under physical conditions found in Seyfert nuclei, 14 of 70 transitions examined have significant population inversions in levels that give rise to IR coronal lines. Several IR coronal line transitions were found to have laser gain lengths that correspond to column densities of 10 exp 24-25/sq cm which are modeled to exist in Seyfert nuclei. Observations that can reveal inverted level populations and laser gain in IR coronal lines are suggested.

  16. High-order above-threshold dissociation of molecules

    NASA Astrophysics Data System (ADS)

    Lu, Peifen; Wang, Junping; Li, Hui; Lin, Kang; Gong, Xiaochun; Song, Qiying; Ji, Qinying; Zhang, Wenbin; Ma, Junyang; Li, Hanxiao; Zeng, Heping; He, Feng; Wu, Jian

    2018-03-01

    Electrons bound to atoms or molecules can simultaneously absorb multiple photons via the above-threshold ionization featured with discrete peaks in the photoelectron spectrum on account of the quantized nature of the light energy. Analogously, the above-threshold dissociation of molecules has been proposed to address the multiple-photon energy deposition in the nuclei of molecules. In this case, nuclear energy spectra consisting of photon-energy spaced peaks exceeding the binding energy of the molecular bond are predicted. Although the observation of such phenomena is difficult, this scenario is nevertheless logical and is based on the fundamental laws. Here, we report conclusive experimental observation of high-order above-threshold dissociation of H2 in strong laser fields where the tunneling-ionized electron transfers the absorbed multiphoton energy, which is above the ionization threshold to the nuclei via the field-driven inelastic rescattering. Our results provide an unambiguous evidence that the electron and nuclei of a molecule as a whole absorb multiple photons, and thus above-threshold ionization and above-threshold dissociation must appear simultaneously, which is the cornerstone of the nowadays strong-field molecular physics.

  17. Probing Long-Range Neutrino-Mediated Forces with Atomic and Nuclear Spectroscopy.

    PubMed

    Stadnik, Yevgeny V

    2018-06-01

    The exchange of a pair of low-mass neutrinos between electrons, protons, and neutrons produces a "long-range" 1/r^{5} potential, which can be sought for in phenomena originating on the atomic and subatomic length scales. We calculate the effects of neutrino-pair exchange on transition and binding energies in atoms and nuclei. In the case of atomic s-wave states, there is a large enhancement of the induced energy shifts due to the lack of a centrifugal barrier and the highly singular nature of the neutrino-mediated potential. We derive limits on neutrino-mediated forces from measurements of the deuteron binding energy and transition energies in positronium, muonium, hydrogen, and deuterium, as well as isotope-shift measurements in calcium ions. Our limits improve on existing constraints on neutrino-mediated forces from experiments that search for new macroscopic forces by 18 orders of magnitude. Future spectroscopy experiments have the potential to probe long-range forces mediated by the exchange of pairs of standard-model neutrinos and other weakly charged particles.

  18. Probing Long-Range Neutrino-Mediated Forces with Atomic and Nuclear Spectroscopy

    NASA Astrophysics Data System (ADS)

    Stadnik, Yevgeny V.

    2018-06-01

    The exchange of a pair of low-mass neutrinos between electrons, protons, and neutrons produces a "long-range" 1 /r5 potential, which can be sought for in phenomena originating on the atomic and subatomic length scales. We calculate the effects of neutrino-pair exchange on transition and binding energies in atoms and nuclei. In the case of atomic s -wave states, there is a large enhancement of the induced energy shifts due to the lack of a centrifugal barrier and the highly singular nature of the neutrino-mediated potential. We derive limits on neutrino-mediated forces from measurements of the deuteron binding energy and transition energies in positronium, muonium, hydrogen, and deuterium, as well as isotope-shift measurements in calcium ions. Our limits improve on existing constraints on neutrino-mediated forces from experiments that search for new macroscopic forces by 18 orders of magnitude. Future spectroscopy experiments have the potential to probe long-range forces mediated by the exchange of pairs of standard-model neutrinos and other weakly charged particles.

  19. Quantum self-organization and nuclear collectivities

    NASA Astrophysics Data System (ADS)

    Otsuka, T.; Tsunoda, Y.; Togashi, T.; Shimizu, N.; Abe, T.

    2018-02-01

    The quantum self-organization is introduced as one of the major underlying mechanisms of the quantum many-body systems. In the case of atomic nuclei as an example, two types of the motion of nucleons, single-particle states and collective modes, dominate the structure of the nucleus. The outcome of the collective mode is determined basically by the balance between the effect of the mode-driving force (e.g., quadrupole force for the ellipsoidal deformation) and the resistance power against it. The single-particle energies are one of the sources to produce such resistance power: a coherent collective motion is more hindered by larger gaps between relevant single particle states. Thus, the single-particle state and the collective mode are “enemies” each other. However, the nuclear forces are demonstrated to be rich enough so as to enhance relevant collective mode by reducing the resistance power by changing singleparticle energies for each eigenstate through monopole interactions. This will be verified with the concrete example taken from Zr isotopes. Thus, when the quantum self-organization occurs, single-particle energies can be self-organized, being enhanced by (i) two quantum liquids, e.g., protons and neutrons, (ii) two major force components, e.g., quadrupole interaction (to drive collective mode) and monopole interaction (to control resistance). In other words, atomic nuclei are not necessarily like simple rigid vases containing almost free nucleons, in contrast to the naïve Fermi liquid picture. Type II shell evolution is considered to be a simple visible case involving excitations across a (sub)magic gap. The quantum self-organization becomes more important in heavier nuclei where the number of active orbits and the number of active nucleons are larger. The quantum self-organization is a general phenomenon, and is expected to be found in other quantum systems.

  20. Hyperspectral microscopic analysis of normal, benign and carcinoma microarray tissue sections

    NASA Astrophysics Data System (ADS)

    Maggioni, Mauro; Davis, Gustave L.; Warner, Frederick J.; Geshwind, Frank B.; Coppi, Andreas C.; DeVerse, Richard A.; Coifman, Ronald R.

    2006-02-01

    We apply a unique micro-optoelectromechanical tuned light source and new algorithms to the hyper-spectral microscopic analysis of human colon biopsies. The tuned light prototype (Plain Sight Systems Inc.) transmits any combination of light frequencies, range 440nm 700nm, trans-illuminating H and E stained tissue sections of normal (N), benign adenoma (B) and malignant carcinoma (M) colon biopsies, through a Nikon Biophot microscope. Hyper-spectral photomicrographs, randomly collected 400X magnication, are obtained with a CCD camera (Sensovation) from 59 different patient biopsies (20 N, 19 B, 20 M) mounted as a microarray on a single glass slide. The spectra of each pixel are normalized and analyzed to discriminate among tissue features: gland nuclei, gland cytoplasm and lamina propria/lumens. Spectral features permit the automatic extraction of 3298 nuclei with classification as N, B or M. When nuclei are extracted from each of the 59 biopsies the average classification among N, B and M nuclei is 97.1%; classification of the biopsies, based on the average nuclei classification, is 100%. However, when the nuclei are extracted from a subset of biopsies, and the prediction is made on nuclei in the remaining biopsies, there is a marked decrement in performance to 60% across the 3 classes. Similarly the biopsy classification drops to 54%. In spite of these classification differences, which we believe are due to instrument and biopsy normalization issues, hyper-spectral analysis has the potential to achieve diagnostic efficiency needed for objective microscopic diagnosis.

  1. OH+ and H2O+: Probes of the Molecular Hydrogen Fraction and Cosmic-Ray Ionization Rate

    NASA Astrophysics Data System (ADS)

    Indriolo, Nick; Neufeld, D. A.; Gerin, M.; PRISMAS; WISH

    2014-01-01

    The fast ion-molecule chemistry that occurs in the interstellar medium (ISM) is initiated by cosmic-ray ionization of both atomic and molecular hydrogen. Species that are near the beginning of the network of interstellar chemistry such as the oxygen-bearing ions OH+ and H2O+ can be useful probes of the cosmic-ray ionization rate. This parameter is of particular interest as, to some extent, it controls the abundances of several molecules. Using observations of OH+ and H2O+ made with HIFI on board Herschel, we have inferred the cosmic-ray ionization rate of atomic hydrogen in multiple distinct clouds along 12 Galactic sight lines. These two molecules also allow us to determine the molecular hydrogen fraction (amount of hydrogen nuclei in H2 versus H) as OH+ and H2O+ abundances are dependent on the competition between dissociative recombination with electrons and hydrogen abstraction reactions involving H2. Our observations of OH+ and H2O+ indicate environments where H2 accounts for less than 10% of the available hydrogen nuclei, suggesting that these species primarily reside in the diffuse, atomic ISM. Average ionization rates in this gas are on the order of a few times 10-16 s-1, with most values in specific clouds above or below this average by a factor of 3 or so. This result is in good agreement with the most up-to-date determination of the distribution of cosmic-ray ionization rates in diffuse molecular clouds as inferred from observations of H3+.

  2. Pressure dependence of side chain 13C chemical shifts in model peptides Ac-Gly-Gly-Xxx-Ala-NH2.

    PubMed

    Beck Erlach, Markus; Koehler, Joerg; Crusca, Edson; Munte, Claudia E; Kainosho, Masatsune; Kremer, Werner; Kalbitzer, Hans Robert

    2017-10-01

    For evaluating the pressure responses of folded as well as intrinsically unfolded proteins detectable by NMR spectroscopy the availability of data from well-defined model systems is indispensable. In this work we report the pressure dependence of 13 C chemical shifts of the side chain atoms in the protected tetrapeptides Ac-Gly-Gly-Xxx-Ala-NH 2 (Xxx, one of the 20 canonical amino acids). Contrary to expectation the chemical shifts of a number of nuclei have a nonlinear dependence on pressure in the range from 0.1 to 200 MPa. The size of the polynomial pressure coefficients B 1 and B 2 is dependent on the type of atom and amino acid studied. For H N , N and C α the first order pressure coefficient B 1 is also correlated to the chemical shift at atmospheric pressure. The first and second order pressure coefficients of a given type of carbon atom show significant linear correlations suggesting that the NMR observable pressure effects in the different amino acids have at least partly the same physical cause. In line with this observation the magnitude of the second order coefficients of nuclei being direct neighbors in the chemical structure also are weakly correlated. The downfield shifts of the methyl resonances suggest that gauche conformers of the side chains are not preferred with pressure. The valine and leucine methyl groups in the model peptides were assigned using stereospecifically 13 C enriched amino acids with the pro-R carbons downfield shifted relative to the pro-S carbons.

  3. Nuclear Matter Properties with the Re-evaluated Coefficients of Liquid Drop Model

    NASA Astrophysics Data System (ADS)

    Chowdhury, P. Roy; Basu, D. N.

    2006-06-01

    The coefficients of the volume, surface, Coulomb, asymmetry and pairing energy terms of the semiempirical liquid drop model mass formula have been determined by furnishing best fit to the observed mass excesses. Slightly different sets of the weighting parameters for liquid drop model mass formula have been obtained from minimizations of \\chi 2 and mean square deviation. The most recent experimental and estimated mass excesses from Audi-Wapstra-Thibault atomic mass table have been used for the least square fitting procedure. Equation of state, nuclear incompressibility, nuclear mean free path and the most stable nuclei for corresponding atomic numbers, all are in good agreement with the experimental results.

  4. Bigger Brains or Bigger Nuclei? Regulating the Size of Auditory Structures in Birds

    PubMed Central

    Kubke, M. Fabiana; Massoglia, Dino P.; Carr, Catherine E.

    2012-01-01

    Increases in the size of the neuronal structures that mediate specific behaviors are believed to be related to enhanced computational performance. It is not clear, however, what developmental and evolutionary mechanisms mediate these changes, nor whether an increase in the size of a given neuronal population is a general mechanism to achieve enhanced computational ability. We addressed the issue of size by analyzing the variation in the relative number of cells of auditory structures in auditory specialists and generalists. We show that bird species with different auditory specializations exhibit variation in the relative size of their hindbrain auditory nuclei. In the barn owl, an auditory specialist, the hind-brain auditory nuclei involved in the computation of sound location show hyperplasia. This hyperplasia was also found in songbirds, but not in non-auditory specialists. The hyperplasia of auditory nuclei was also not seen in birds with large body weight suggesting that the total number of cells is selected for in auditory specialists. In barn owls, differences observed in the relative size of the auditory nuclei might be attributed to modifications in neurogenesis and cell death. Thus, hyperplasia of circuits used for auditory computation accompanies auditory specialization in different orders of birds. PMID:14726625

  5. A-dependence of phi meson production at HERA-B

    NASA Astrophysics Data System (ADS)

    Ispiryan, Mikayel

    In the HERA-B experiment at DESY, Germany, 920 GeV protons collide with nuclei of the targets. In the collisions many hadrons are produced and detected by the spectrometer, allowing the study of various issues of hadron-hadron and hadron-nucleus interactions. In this thesis the production dependence of the φ meson on the atomic weight A of the nuclei has been studied for several materials, with the goal of obtaining experimental information on proton-nucleus (p-A) interactions. For this, runs and events have been selected according to special criteria. The φ meson's signature---its decay into two charged kaons---has been used to detect the fact of the production of a φ meson in the collision. The RICH detector, the tracking system, and selection algorithms have been used for identification of kaons. The main result, obtaining of which does not depend on the knowledge of integrated luminosity and does not depend heavily on the Monte Carlo simulation of the spectrometer, is the exponent Deltaalpha of the power law of the φ meson production cross-section in an inelastic interaction: sigma ∝ ADeltaalpha, which was measured to be 0.14 .. 0.19 for tungsten, titanium and rhenium, with Deltaalpha = 0.141 +/- 0.012(stat) +/- 0.022(sys) being the most exact number obtained from the analysis of ˜108 events on carbon and tungsten targets. As a by-product, the mass of the φ meson is obtained to be 1.01957 GeV, which did not show dependence on the type of the target nucleus within statistical error of approximately +/-80 keV. The results show a clear experimental indication of A-dependence for φ meson production in proton-nucleon inelastic interactions.

  6. Electron-Molecule Col1isions: Quantitative Approaches, and the Legacy of Aaron Temkin

    NASA Technical Reports Server (NTRS)

    Schneider, B.I.

    2007-01-01

    This article, on electron-molecule collisions, is dedicated to the legacy of my good friend and sometime collaborator, Aaron Temkin on his retirement from the NASA-Goddard Space Flight Center after many years of work at the highest intellectual level in the theoretical treatment of electron-atom and electron-molecule scattering. Aaron's contributions to the manner in which we think about electron-molecule collisions is clear to all of us who have worked in this field. I doubt that the great progress that has occurred in the computational treatment of such complex collision problems could have happened without these contributions. For a brief historical account, see the discussion of Temkin's contribution to electron-molecule scattering in the first article of this volume by Dr. A. K. Bhatia. In this article, I will concentrate on the application of the so called, non-adiabatic R-matrix theory, to vibrational excitation and dissociative attachment, although I will also present some results applying the Linear Algebraic and Kohn-Variational methods to vibrational excitation. As a starting point for almost all computationally effective approaches to electron-molecule collisions, is the fixed nuclei approximation. That is, one recognizes, just as one does with molecular bound states, that there is a separation of electronic(fast) and nuclear(s1ow) degrees of freedom. This separation makes it possible to "freeze" the nuclei in space, calculate the collision parameters for the frozen molecule and then, somehow to add back the vibrations and rotations. The manner in which this is done, depends on the details of the collision problem. It is the work of Aaron and a number of other researchers that has provided the guidance necessary to resolve these issues.

  7. Theory of electronic structures and nuclear quadrupole interactions in molecular solids and semiconductor surfaces

    NASA Astrophysics Data System (ADS)

    Pati, Ranjit

    We have investigated, using the Hartree-Fock Roothaan variational procedure, the electronic structures and associated nuclear quadrupole interactions (NQI) for the molecular solids, RDX (C3H6N6O6),/ /beta- HMX(C4H8N8O8), Cocaine (C17H21NO4), Cocaine Hydrochloride (C17H21NO4HCl) and Heroin (C21H23NO5) and for the (111) surface of silicon with adsorbed radioactive 111In atom and negative cadmium ion containing the excited nucleus 111Cd/* resulting from electron capture by lllIn. Our investigations indicate that for the ring 14N NQI parameters in RDX and β-HMX there is very good agreement between theory and experiment. For the peripheral 14N nuclei in NO2 groups, while the calculated electronic structures do explain the much weaker quadrupole coupling constants for these nuclei relative to the ring 14N nuclei, there are significant differences between theory and experiment. The influence of intermolecular interactions between adjacent molecules in the solid is invoked as a possible source for these differences. For the controlled substances, Cocaine and Heroin, again very good agreement is obtained between theory and experiment. For Cocaine Hydrochloride theory is able to explain the much smaller observed 14N nuclear quadrupole resonance frequency as compared to pure Cocaine. However there are significant differences between theory and experiment for the 14N and 35Cl quadrupole resonance frequencies. The influence of intermolecular interactions is one of the factors suggested to explain the difference. For the silicon (111) surface, the observed 111Cd/* NQI parameters, with the cadmium nucleus assumed to be located at the same site as the 111In nucleus from which it is generated, can be successfully explained by theory with the indium atom located at the two distinct sites available with the DAS model for the 7 x 7 reconstructed (111) surface. Some quantitative differences still remain, one of the main factor suggested for their explanation being a need for a thorough analysis of relaxation effects in the positions of silicon atoms associated with the presence of the indium atom. Applications of the Hartree-Fock Cluster theory to other related systems is suggested to subject the DAS model to additional tests at the microscopic level as in the system studied in the present thesis. (Abstract shortened by UMI.)

  8. Combining X-ray and neutron crystallography with spectroscopy.

    PubMed

    Kwon, Hanna; Smith, Oliver; Raven, Emma Lloyd; Moody, Peter C E

    2017-02-01

    X-ray protein crystallography has, through the determination of the three-dimensional structures of enzymes and their complexes, been essential to the understanding of biological chemistry. However, as X-rays are scattered by electrons, the technique has difficulty locating the presence and position of H atoms (and cannot locate H + ions), knowledge of which is often crucially important for the understanding of enzyme mechanism. Furthermore, X-ray irradiation, through photoelectronic effects, will perturb the redox state in the crystal. By using single-crystal spectrophotometry, reactions taking place in the crystal can be monitored, either to trap intermediates or follow photoreduction during X-ray data collection. By using neutron crystallography, the positions of H atoms can be located, as it is the nuclei rather than the electrons that scatter neutrons, and the scattering length is not determined by the atomic number. Combining the two techniques allows much greater insight into both reaction mechanism and X-ray-induced photoreduction.

  9. Electron quantum dynamics in atom-ion interaction

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Sabzyan, H., E-mail: sabzyan@sci.ui.ac.ir; Jenabi, M. J.

    2016-04-07

    Electron transfer (ET) process and its dependence on the system parameters are investigated by solving two-dimensional time-dependent Schrödinger equation numerically using split operator technique. Evolution of the electron wavepacket occurs from the one-electron species hydrogen atom to another bare nucleus of charge Z > 1. This evolution is quantified by partitioning the simulation box and defining regional densities belonging to the two nuclei of the system. It is found that the functional form of the time-variations of these regional densities and the extent of ET process depend strongly on the inter-nuclear distance and relative values of the nuclear charges, whichmore » define the potential energy surface governing the electron wavepacket evolution. Also, the initial electronic state of the single-electron atom has critical effect on this evolution and its consequent (partial) electron transfer depending on its spreading extent and orientation with respect to the inter-nuclear axis.« less

  10. Morphology and force probing of primary murine liver sinusoidal endothelial cells.

    PubMed

    Zapotoczny, B; Owczarczyk, K; Szafranska, K; Kus, E; Chlopicki, S; Szymonski, M

    2017-07-01

    Liver sinusoidal endothelial cells (LSECs) represent unique type of endothelial cells featured by their characteristic morphology, ie, lack of a basement membrane and presence of fenestrations-transmembrane pores acting as a dynamic filter between the vascular space and the liver parenchyma. Delicate structure of LSECs membrane combined with a submicron size of fenestrations hinders their visualization in live cells. In this work, we apply atomic force microscopy contact mode to characterize fenestrations in LSECs. We reveal the structure of fenestrations in live LSECs. Moreover, we show that the high-resolution imaging of fenestrations is possible for the glutaraldehyde-fixed LSECs. Finally, thorough information about the morphology of LSECs including great contrast in visualization of sieve plates and fenestrations is provided using Force Modulation mode. We show also the ability to precisely localize the cell nuclei in fixed LSECs. It can be helpful for more precise description of nanomechanical properties of cell nuclei using atomic force microscopy. Presented methodology combining high-quality imaging of fixed cells with an additional nanomechanical information of both live and fixed LSECs provides a unique approach to study LSECs morphology and nanomechanics that could foster understanding of the role of LSECs in maintaining liver homeostasis. Copyright © 2017 John Wiley & Sons, Ltd.

  11. Neutron production by cosmic-ray muons in various materials

    NASA Astrophysics Data System (ADS)

    Manukovsky, K. V.; Ryazhskaya, O. G.; Sobolevsky, N. M.; Yudin, A. V.

    2016-07-01

    The results obtained by studying the background of neutrons produced by cosmic-raymuons in underground experimental facilities intended for rare-event searches and in surrounding rock are presented. The types of this rock may include granite, sedimentary rock, gypsum, and rock salt. Neutron production and transfer were simulated using the Geant4 and SHIELD transport codes. These codes were tuned via a comparison of the results of calculations with experimental data—in particular, with data of the Artemovsk research station of the Institute for Nuclear Research (INR, Moscow, Russia)—as well as via an intercomparison of results of calculations with the Geant4 and SHIELD codes. It turns out that the atomic-number dependence of the production and yield of neutrons has an irregular character and does not allow a description in terms of a universal function of the atomic number. The parameters of this dependence are different for two groups of nuclei—nuclei consisting of alpha particles and all of the remaining nuclei. Moreover, there are manifest exceptions from a power-law dependence—for example, argon. This may entail important consequences both for the existing underground experimental facilities and for those under construction. Investigation of cosmic-ray-induced neutron production in various materials is of paramount importance for the interpretation of experiments conducted at large depths under the Earth's surface.

  12. Temperature dependence of stacking faults in catalyst-free GaAs nanopillars.

    PubMed

    Shapiro, Joshua N; Lin, Andrew; Ratsch, Christian; Huffaker, D L

    2013-11-29

    Impressive opto-electronic devices and transistors have recently been fabricated from GaAs nanopillars grown by catalyst-free selective-area epitaxy, but this growth technique has always resulted in high densities of stacking faults. A stacking fault occurs when atoms on the growing (111) surface occupy the sites of a hexagonal-close-pack (hcp) lattice instead of the normal face-centered-cubic (fcc) lattice sites. When stacking faults occur consecutively, the crystal structure is locally wurtzite instead of zinc-blende, and the resulting band offsets are known to negatively impact device performance. Here we present experimental and theoretical evidence that indicate stacking fault formation is related to the size of the critical nucleus, which is temperature dependent. The difference in energy between the hcp and fcc orientation of small nuclei is computed using density-function theory. The minimum energy difference of 0.22 eV is calculated for a nucleus with 21 atoms, so the population of nuclei in the hcp orientation is expected to decrease as the nucleus grows larger. The experiment shows that stacking fault occurrence is dramatically reduced from 22% to 3% by raising the growth temperature from 730 to 790 ° C. These data are interpreted using classical nucleation theory which dictates a larger critical nucleus at higher growth temperature.

  13. New Mechanism of Low Energy Nuclear Reactions Using Superlow

    NASA Astrophysics Data System (ADS)

    Gareev, F. A.; Zhidkova, I. E.

    2006-03-01

    We proposed a new mechanism of LENR (low energy nuclear reactions) cooperative processes in the whole system - nuclei+atoms+condensed matter can occur at smaller threshold than the corresponding ones assoiciated with free constituents. The cooperative processes can be induced and enhanced by (``superlow energy'') external fields. The excess heat is the emission of internal energy, and transmutations from LENR are the result of redistribution of the internal energy of the whole system. A review of possible stimulation mechanisms of LENR is presented. We have concluded that transmutation of nuclei at low energies and excess heat are possible in the framework of the known fundamental physical laws: The universal resonance synchronization principle, and based on it, different enhancement mechanisms of reaction rates are responsible for these processes. The excitation and ionization of atoms may play the role of a trigger for LENR. F.A. Gareev, I.E. Zhidkova, E-print arXiv Nucl-th/0511092 v1 30 Nov 2005. F.A. Gareev, In: FPB-98, Novosibirsk, June 1998, p.92; F.A.Gareev, G.F. Gareeva, in: Novosibirsk, July 2000, p.161. F.A. Gareev, I.E. Zhidkova and Yu.L. Ratis, Preprint JINR P4-2004-68, Dubna, 2004. F.A. Gareev, I.E. Zhidkova, E-print arXiv Nucl-th/0505021 9 May 2005.

  14. Understanding the crystallization behavior of as-deposited Ti-Sb-Te alloys through real-time radial distribution functions.

    PubMed

    Zhu, Min; Xia, Mengjiao; Song, Zhitang; Cheng, Yan; Wu, Liangcai; Rao, Feng; Song, Sannian; Wang, Miao; Lu, Yegang; Feng, Songlin

    2015-06-07

    Phase change materials, successfully used in optical data-storage and non-volatile electronic memory, are well-known for their ultrafast crystallization speed. However, the fundamental understanding of their crystallization behavior, especially the nucleation process, is limited by present experimental techniques. Here, real-time radial distribution functions (RDFs), derived from the selected area electron diffractions, are employed as structural probes to comprehensively study both nucleation and subsequent growth stages of Ti-doped Sb2Te3 (TST) materials in the electron-irradiation crystallization process. It can be found that the incorporation of Ti atoms in Sb2Te3 forms wrong bonds such as Ti-Te, Ti-Sb, breaks the originally ordered atomic arrangement and diminishes the initial nucleus size of the as-deposited films, which results in better thermal stability. But these nuclei hardly grow until their sizes exceed a critical value, and then a rapid growth period starts. This means that an extended nucleation time is required to form the supercritical nuclei of TST alloys with higher concentration. Also, the increasing formation of four-membered rings, which served as nucleation sites, after doping excessive Ti is responsible for the change of the crystallization behavior from growth-dominated to nucleation-dominated.

  15. Search For ɛ-Bound Nuclei

    NASA Astrophysics Data System (ADS)

    Machner, H.

    2011-10-01

    The η meson can be bound to atomic nuclei. Experimental search is discussed in the form of final state interaction for the reactions dp→3Heη and dd→4Heη. For the latter case tensor polarized deuterons were used in order to extract the s-wave strength. For both reactions complex scattering lengths are deduced: In a two-nucleon transfer reaction under quasi-free conditions, p27Al→3HeX, was investigated. The system X can be the bound 25Mg⊗η at rest. When a possible decay of an intermediate N*(1535) is required, a highly significant bump shows up in the missing mass spectrum. The data give for a bound state a binding energy of 13.3±1.6 MeV and a width of σ = 4.4±1.3 MeV.

  16. Nuclear Physics Around the Unitarity Limit

    DOE PAGES

    König, Sebastian; Grießhammer, Harald W.; Hammer, H. -W.; ...

    2017-05-15

    We argue that many features of the structure of nuclei emerge from a strictly perturbative expansion around the unitarity limit, where the two-nucleon S waves have bound states at zero energy. In this limit, the gross features of states in the nuclear chart are correlated to only one dimensionful parameter, which is related to the breaking of scale invariance to a discrete scaling symmetry and set by the triton binding energy. Observables are moved to their physical values by small perturbative corrections, much like in descriptions of the fine structure of atomic spectra. We provide evidence in favor of themore » conjecture that light, and possibly heavier, nuclei are bound weakly enough to be insensitive to the details of the interactions but strongly enough to be insensitive to the exact size of the two-nucleon system.« less

  17. Cosmic-ray energy spectra between 10 and several hundred GeV per atomic mass unit for elements from Ar-18 to Ni-28 - Results from HEAO 3

    NASA Technical Reports Server (NTRS)

    Binns, W. R.; Israel, M. H.; Jones, Michael D.; Kamionkowski, M. P.; Garrard, T. L.

    1988-01-01

    Results from the Heavy Nuclei experiment on HEAO 3 are used to determine the primary abundances of Ni and Fe. Ni and Fe are found to have nearly constant relative abundances over the interval of 10 to about 500 GeV per amu. Individual secondary elements derived principally from interactions of primary Fe nuclei are shown to display a power-law decrease in relative abundance up to about 150 GeV per amu. Ar/Fe and Ca/Fe ratios of 2.6 + or - 0.7 percent and 8.8 + or - 0.7 percent, respectively, are found, confirming a fractionation of source abundances in which elements with high values of the first ionization potential are depleted relative to those with low first ionization potential.

  18. DAMQT: A package for the analysis of electron density in molecules

    NASA Astrophysics Data System (ADS)

    López, Rafael; Rico, Jaime Fernández; Ramírez, Guillermo; Ema, Ignacio; Zorrilla, David

    2009-09-01

    DAMQT is a package for the analysis of the electron density in molecules and the fast computation of the density, density deformations, electrostatic potential and field, and Hellmann-Feynman forces. The method is based on the partition of the electron density into atomic fragments by means of a least deformation criterion. Each atomic fragment of the density is expanded in regular spherical harmonics times radial factors, which are piecewise represented in terms of analytical functions. This representation is used for the fast evaluation of the electrostatic potential and field generated by the electron density and nuclei, as well as for the computation of the Hellmann-Feynman forces on the nuclei. An analysis of the atomic and molecular deformations of the density can be also carried out, yielding a picture that connects with several concepts of the empirical structural chemistry. Program summaryProgram title: DAMQT1.0 Catalogue identifier: AEDL_v1_0 Program summary URL:http://cpc.cs.qub.ac.uk/summaries/AEDL_v1_0.html Program obtainable from: CPC Program Library, Queen's University, Belfast, N. Ireland Licensing provisions: GPLv3 No. of lines in distributed program, including test data, etc.: 278 356 No. of bytes in distributed program, including test data, etc.: 31 065 317 Distribution format: tar.gz Programming language: Fortran90 and C++ Computer: Any Operating system: Linux, Windows (Xp, Vista) RAM: 190 Mbytes Classification: 16.1 External routines: Trolltech's Qt (4.3 or higher) ( http://www.qtsoftware.com/products), OpenGL (1.1 or higher) ( http://www.opengl.org/), GLUT 3.7 ( http://www.opengl.org/resources/libraries/glut/). Nature of problem: Analysis of the molecular electron density and density deformations, including fast evaluation of electrostatic potential, electric field and Hellmann-Feynman forces on nuclei. Solution method: The method of Deformed Atoms in Molecules, reported elsewhere [1], is used for partitioning the molecular electron density into atomic fragments, which are further expanded in spherical harmonics times radial factors. The partition is used for defining molecular density deformations and for the fast calculation of several properties associated to density. Restrictions: The current version is limited to 120 atoms, 2000 contracted functions, and l=5 in basis functions. Density must come from a LCAO calculation (any level) with spherical (not Cartesian) Gaussian functions. Unusual features: The program contains an OPEN statement to binary files (stream) in file GOPENMOL.F90. This statement has not a standard syntax in Fortran 90. Two possibilities are considered in conditional compilation: Intel's ifort and Fortran2003 standard. This latter is applied to compilers other than ifort (gfortran uses this one, for instance). Additional comments: The distribution file for this program is over 30 Mbytes and therefore is not delivered directly when download or e-mail is requested. Instead a html file giving details of how the program can be obtained is sent. Running time: Largely dependent on the system size and the module run (from fractions of a second to hours). References: [1] J. Fernández Rico, R. López, I. Ema, G. Ramírez, J. Mol. Struct. (Theochem) 727 (2005) 115.

  19. Development of a collinear laser spectrometer facility at VECC: First test result

    NASA Astrophysics Data System (ADS)

    Ali, Md Sabir; Ray, Ayan; Raja, Waseem; Bandyopadhyay, Arup; Naik, Vaishali; Polley, Asish; Chakrabarti, Alok

    2018-04-01

    We report here the development of collinear laser spectroscopy (CLS) system at VECC for the study of hyperfine spectrum and isotopic shift of stable and unstable isotopes. The facility is first of its kind in the country allowing measurement of hyperfine splitting of atomic levels using atomic beams. The CLS system is installed downstream of the focal plane of the existing isotope separator online (ISOL) facility at VECC and is recently commissioned by successfully resolving the fluorescence spectrum of the hyperfine levels in ^{85,87}Rb. The atomic beams of Rb were produced by charge exchange of 8 keV Rb ion beam which were produced, extracted and transported to the charge exchange cell using the ion sources, extractor and the beam-line magnets of the ISOL facility. The laser propagating opposite to the ion / atom beam direction was allowed to interact with the atom beam and fluorescence spectrum was recorded. The experimental set-up and the experiment conducted are reported in detail. The measures needed to be carried out for improving the sensitivity to a level necessary for studying short-lived exotic nuclei have also been discussed.

  20. Ultrasonic atomization of tissue and its role in tissue fractionation by high intensity focused ultrasound

    PubMed Central

    Simon, Julianna C.; Sapozhnikov, Oleg A.; Khokhlova, Vera A.; Wang, Yak-Nam; Crum, Lawrence A.; Bailey, Michael R.

    2012-01-01

    Atomization and fountain formation is a well-known phenomenon that occurs when a focused ultrasound wave in liquid encounters an air interface. High intensity focused ultrasound (HIFU) has been shown to fractionate tissue into submicron-size fragments in a process termed boiling histotripsy, wherein the focused ultrasound wave superheats the tissue at the focus, producing a millimetre-size boiling or vapour bubble in several milliseconds. Yet the question of how this millimetre-size boiling bubble creates submicron-size tissue fragments remains. The hypothesis of this work is that tissue can behave as a liquid such that it forms a fountain and atomization within the vapour bubble produced in boiling histotripsy. We describe an experiment, in which a 2-MHz HIFU transducer (maximum in situ intensity of 24,000 W/cm2) was aligned with an air-tissue interface meant to simulate the boiling bubble. Atomization and fountain formation were observed with high-speed photography and resulted in tissue erosion. Histological examination of the atomized tissue showed whole and fragmented cells and nuclei. Air-liquid interfaces were also filmed. Our conclusion was that HIFU can fountain and atomize tissue. Although this process does not entirely mimic what was observed in liquids, it does explain many aspects of tissue fractionation in boiling histotripsy. PMID:23159812

  1. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Li, Rong; Wu, Yongquan, E-mail: yqwu@shu.edu.cn; Xiao, Junjiang

    We observed homogeneous nucleation process of supercooled liquid Fe by molecular dynamics simulations. Using bond-orientational order parameters together with Voronoi polyhedron method, we characterized local structure, calculated the volume of Voronoi polyhedra of atoms and identified the structure and density fluctuations. We monitored the formation of nucleus and analyzed its inner structure. The birth and growth of the pre-nucleus and nucleus are accompanied with aggregating and disaggregating processes in the time scale of femtosecond. Only the initial solid-like clusters (ISLC), ranging from 1 to 7 atoms, pop up directly from liquid. The relation between the logarithm of number of clustersmore » and the cluster size was found to be linear for ISLCs and was observed to be parabolic for all solid-like clusters (SLC) due to aggregating and disaggregating effects. The nucleus and pre-nuclei mainly consist of body centered cubic (BCC) and hexagonal close packed atoms, while the BCC atoms tend to be located at the surface. Medium-range structure fluctuations induce the birth of ISLCs, benefit the aggregation of embryos and remarkably promote the nucleation. But density fluctuations contribute little to nucleation. The lifetime of most icosahedral-like atoms (ICO) is shorter than 0.7 ps. No obvious relationship was found between structure/density fluctuations and the appearance of ICO atoms.« less

  2. Transition between nuclear and quark-gluon descriptions of hadrons and light nuclei

    NASA Astrophysics Data System (ADS)

    Holt, R. J.; Gilman, R.

    2012-08-01

    We provide a perspective on studies aimed at observing the transition between hadronic and quark-gluonic descriptions of reactions involving light nuclei. We begin by summarizing the results for relatively simple reactions such as the pion form factor and the neutral pion transition form factor as well as that for the nucleon and end with exclusive photoreactions in our simplest nuclei. A particular focus will be on reactions involving the deuteron. It is noted that a firm understanding of these issues is essential for unravelling important structure information from processes such as deeply virtual Compton scattering as well as deeply virtual meson production. The connection to exotic phenomena such as color transparency will be discussed. A number of outstanding challenges will require new experiments at modern facilities on the horizon as well as further theoretical developments.

  3. The complex pericentriolar material 1 protein allows differentiation between myonuclei and nuclei of satellite cells of the skeletal muscle.

    PubMed

    Brunn, Anna

    2018-05-27

    The original article by Winje et al., entitled "Specific labelling of myonuclei by an antibody against pericentriolar material 1 (PCM1) on skeletal muscle tissue sections" 1 , sheds new light on the issue of heterogeneity of skeletal muscle and, thus, the problem to reliably distinguish between myonuclei versus nuclei of satellite cells of the skeletal muscle which are intimately associated. At the light microscopical level this differentiation is particularly difficult since only nuclei inside the muscle fiber are defined as true myonuclei. This is a major problem in analyses that use tissue homogenates, while in situ immunohistochemical studies using appropriate antibodies usually allow differentiation of cell populations. This article is protected by copyright. All rights reserved. This article is protected by copyright. All rights reserved.

  4. Current Status of Nuclear Physics Research

    NASA Astrophysics Data System (ADS)

    Bertulani, Carlos A.; Hussein, Mahir S.

    2015-12-01

    In this review, we discuss the current status of research in nuclear physics which is being carried out in different centers in the world. For this purpose, we supply a short account of the development in the area which evolved over the last nine decades, since the discovery of the neutron. The evolution of the physics of the atomic nucleus went through many stages as more data became available. We briefly discuss models introduced to discern the physics behind the experimental discoveries, such as the shell model, the collective model, the statistical model, the interacting boson model, etc., some of these models may be seemingly in conflict with each other, but this was shown to be only apparent. The richness of the ideas and abundance of theoretical models attests to the important fact that the nucleus is a really singular system in the sense that it evolves from two-body bound states such as the deuteron, to few-body bound states, such as 4He, 7Li, 9Be, etc. and up the ladder to heavier bound nuclei containing up to more than 200 nucleons. Clearly, statistical mechanics, usually employed in systems with very large number of particles, would seemingly not work for such finite systems as the nuclei, neither do other theories which are applicable to condensed matter. The richness of nuclear physics stems from these restrictions. New theories and models are presently being developed. Theories of the structure and reactions of neutron-rich and proton-rich nuclei, called exotic nuclei, halo nuclei, or Borromean nuclei, deal with the wealth of experimental data that became available in the last 35 years. Furthermore, nuclear astrophysics and stellar and Big Bang nucleosynthesis have become a more mature subject. Due to limited space, this review only covers a few selected topics, mainly those with which the authors have worked on. Our aimed potential readers of this review are nuclear physicists and physicists in other areas, as well as graduate students interested in pursuing a career in nuclear physics.

  5. New Cooperative Mechanisms of Low-Energy Nuclear Reactions Using Super Low-Energy External Field

    NASA Astrophysics Data System (ADS)

    Gareev, F. A.; Zhidkova, I. E.

    We propose a new mechanism of LENR: cooperative processes in the whole system, nuclei + atoms + condensed matter, can occur at a smaller threshold energies than the corresponding ones on free constituents. The cooperative processes can be induced and enhanced by low-energy external fields. The excess heat is the emission of internal energy and transmutations at LENR are the result of redistribution of inner energy of the whole system.

  6. Progress in Visualizing Atomic Size Effects with DFT-Chemical Pressure Analysis: From Isolated Atoms to Trends in AB5 Intermetallics.

    PubMed

    Berns, Veronica M; Engelkemier, Joshua; Guo, Yiming; Kilduff, Brandon J; Fredrickson, Daniel C

    2014-08-12

    The notion of atomic size poses an important challenge to chemical theory: empirical evidence has long established that atoms have spatial requirements, which are summarized in tables of covalent, ionic, metallic, and van der Waals radii. Considerations based on these radii play a central role in the design and interpretation of experiments, but few methods are available to directly support arguments based on atomic size using electronic structure methods. Recently, we described an approach to elucidating atomic size effects using theoretical calculations: the DFT-Chemical Pressure analysis, which visualizes the local pressures arising in crystal structures from the interactions of atomic size and electronic effects. Using this approach, a variety of structural phenomena in intermetallic phases have already been understood in terms that provide guidance to new synthetic experiments. However, the applicability of the DFT-CP method to the broad range of the structures encountered in the solid state is limited by two issues: (1) the difficulty of interpreting the intense pressure features that appear in atomic core regions and (2) the need to divide space among pairs of interacting atoms in a meaningful way. In this article, we describe general solutions to these issues. In addressing the first issue, we explore the CP analysis of a test case in which no core pressures would be expected to arise: isolated atoms in large boxes. Our calculations reveal that intense core pressures do indeed arise in these virtually pressure-less model systems and allow us to trace the issue to the shifts in the voxel positions relative to atomic centers upon expanding and contracting the unit cell. A compensatory grid unwarping procedure is introduced to remedy this artifact. The second issue revolves around the difficulty of interpreting the pressure map in terms of interatomic interactions in a way that respects the size differences of the atoms and avoids artificial geometrical constraints. In approaching this challenge, we have developed a scheme for allocating the grid pressures to contacts inspired by the Hirshfeld charge analysis. Here, each voxel is allocated to the contact between the two atoms whose free atom electron densities show the largest values at that position. In this way, the differing sizes of atoms are naturally included in the division of space without resorting to empirical radii. The use of the improved DFT-CP method is illustrated through analyses of the applicability of radius ratio arguments to Laves phase structures and the structural preferences of AB5 intermetallics between the CaCu5 and AuBe5 structure types.

  7. Theoretical study of triaxial shapes of neutron-rich Mo and Ru nuclei

    DOE PAGES

    Zhang, C. L.; Bhat, G. H.; Nazarewicz, W.; ...

    2015-09-10

    Here, whether atomic nuclei can possess triaxial shapes at their ground states is still a subject of ongoing debate. According to theory, good prospects for low-spin triaxiality are in the neutron-rich Mo-Ru region. Recently, transition quadrupole moments in rotational bands of even-mass neutron-rich isotopes of molybdenum and ruthenium nuclei have been measured. The new data have provided a challenge for theoretical descriptions invoking stable triaxial deformations. The purpose of this study is to understand experimental data on rotational bands in the neutron-rich Mo-Ru region, we carried out theoretical analysis of moments of inertia, shapes, and transition quadrupole moments of neutron-richmore » even-even nuclei around 110Ru using self-consistent mean-field and shell model techniques. Methods: To describe yrast structures in Mo and Ru isotopes, we use nuclear density functional theory (DFT) with the optimized energy density functional UNEDF0. We also apply triaxial projected shell model (TPSM) to describe yrast and positive-parity, near-yrast band structures. As a result, our self-consistent DFT calculations predict triaxial ground-state deformations in 106,108Mo and 108,110,112Ru and reproduce the observed low-frequency behavior of moments of inertia. As the rotational frequency increases, a negative-gamma structure, associated with the aligned ν(h 11/2) 2 pair, becomes energetically favored. The computed transition quadrupole moments vary with angular momentum, which reflects deformation changes with rotation; those variations are consistent with experiment. The TPSM calculations explain the observed band structures assuming stable triaxial shapes. Lastly, the structure of neutron-rich even-even nuclei around Ru-110 is consistent with triaxial shape deformations. Our DFT and TPSM frameworks provide a consistent and complementary description of experimental data.« less

  8. Neutron-antineutron oscillations in nuclei

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dover, C.B.; Gal, A.; Richard, J.M.

    1983-03-01

    We present calculations of the neutron-antineutron (n-n-bar) annihilation lifetime T in deuterium, /sup 16/O, and /sup 56/Fe in terms of the free-space oscillation time tau/sub n/n-bar. The coupled Schroedinger equations for the n and n-bar wave functions in a nucleus are solved numerically, using a realistic shell-model potential which fits the empirical binding energies of the neu- p tron orbits, and a complex n-bar-nucleus optical potential obtained from fits to p-bar-atom level shifts. Most previous estimates of T in nuclei, which exhibit large variations, are found to be quite inaccurate. When the nuclear-physics aspects of the problem are handled properlymore » (in particular, the finite neutron binding, the nuclear radius, and the surface diffuseness), the results are found to be rather stable with respect to allowable changes in the parameters of the nuclear model. We conclude that experimental limits on T in nuclei can be used to give reasonably precise constraints on tau/sub n/n-bar: T>10/sup 30/ or 10/sup 31/ yr leads to tau/sub n/n-bar>(1.5--2) x 10/sup 7/ or (5--6) x 10/sup 7/ sec, respectively.« less

  9. Frequency Dependence of Electron Spin-lattice Relaxation for Semiquinones in Alcohol Solutions

    PubMed Central

    Elajaili, Hanan B.; Biller, Joshua R.; Eaton, Sandra S.; Eaton, Gareth R.

    2014-01-01

    The spin-lattice relaxation rates at 293 K for three anionic semiquinones (2,5-di-t-butyl-1,4-benzosemiquinone, 2,6-di-t-butyl-1,4-benzosemiquinone, and 2,3,5,6-tetramethoxy-1,4-benzosemiquinone) were studied at up to 8 frequencies between 250 MHz and 34 GHz in ethanol or methanol solution containing high concentrations of OH-. The relaxation rates are about a factor of 2 faster at lower frequencies than at 9 or 34 GHz. However, in perdeuterated alcohols the relaxation rates exhibit little frequency dependence, which demonstrates that the dominant frequency-dependent contribution to relaxation is modulation of dipolar interactions with solvent nuclei. The relaxation rates were modeled as the sum of two frequency-independent contributions (spin rotation and a local mode) and two frequency-dependent contributions (modulation of dipolar interaction with solvent nuclei and a much smaller contribution from modulation of g anisotropy). The correlation time for modulation of the interaction with solvent nuclei is longer than the tumbling correlation time of the semiquinone and is consistent with hydrogen bonding of the alcohol to the oxygen atoms of the semiquinones. PMID:25261741

  10. The physics of spin polarized gases

    NASA Astrophysics Data System (ADS)

    Cates, Gordon D.

    1995-01-01

    Most of our research was connected either directly or indirectly to the study of spin polarized atoms and nuclei, and their applications. In most cases we used lasers to optically pump, and hence polarize, alkali-metal vapors. Spin-exchange collisions were used to transfer the angular momentum to other systems. Of particular interest was our continuing study of the polarization of noble gas nuclei, which are characterized by extremely long spin relaxation times of minutes to many days. During this past research period we have demonstrated several applications of polarized noble gas nuclei that may have important implications for such diverse areas as nondestructive testing and medical diagnostics, as well as many areas in fundamental research. Of particular note is the use of spin-exchange polarized He-3 and Xe-129 for magnetic resonance imaging. At present, our imaging work has focused on the lungs of small animals such as mice and guinea pigs. We believe, however, that our technique would also be useful for nondestructive testing. We have also continued our study of Xe that is polarized in the gaseous state, and subsequently frozen. This novel technique for producing a highly polarized solid has received considerable attention in the NMR community.

  11. High-order above-threshold dissociation of molecules.

    PubMed

    Lu, Peifen; Wang, Junping; Li, Hui; Lin, Kang; Gong, Xiaochun; Song, Qiying; Ji, Qinying; Zhang, Wenbin; Ma, Junyang; Li, Hanxiao; Zeng, Heping; He, Feng; Wu, Jian

    2018-02-27

    Electrons bound to atoms or molecules can simultaneously absorb multiple photons via the above-threshold ionization featured with discrete peaks in the photoelectron spectrum on account of the quantized nature of the light energy. Analogously, the above-threshold dissociation of molecules has been proposed to address the multiple-photon energy deposition in the nuclei of molecules. In this case, nuclear energy spectra consisting of photon-energy spaced peaks exceeding the binding energy of the molecular bond are predicted. Although the observation of such phenomena is difficult, this scenario is nevertheless logical and is based on the fundamental laws. Here, we report conclusive experimental observation of high-order above-threshold dissociation of H 2 in strong laser fields where the tunneling-ionized electron transfers the absorbed multiphoton energy, which is above the ionization threshold to the nuclei via the field-driven inelastic rescattering. Our results provide an unambiguous evidence that the electron and nuclei of a molecule as a whole absorb multiple photons, and thus above-threshold ionization and above-threshold dissociation must appear simultaneously, which is the cornerstone of the nowadays strong-field molecular physics. Copyright © 2018 the Author(s). Published by PNAS.

  12. Many particle spectroscopy of atoms, molecules, clusters and surfaces: international conference MPS-2016

    NASA Astrophysics Data System (ADS)

    Grum-Grzhimailo, Alexei N.; Popov, Yuri V.; Gryzlova, Elena V.; Solov'yov, Andrey V.

    2017-07-01

    The conference on Many Particle Spectroscopy of Atoms, Molecules, Clusters and Surfaces (MPS-2016) brought together near to a hundred scientists in the field of electronic, photonic, atomic and molecular collisions, and spectroscopy from around the world. We deliver an Editorial of a topical issue presenting original research results from some of the participants on both experimental and theoretical studies involving many particle spectroscopy of atoms, molecules, clusters and surfaces. Contribution to the Topical Issue "Many Particle Spectroscopy of Atoms, Molecules, Clusters and Surfaces", edited by A.N. Grum-Grzhimailo, E.V. Gryzlova, Yu.V. Popov, and A.V. Solov'yov.

  13. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Marchenko, A. V.; Terukov, E. I.; Egorova, A. Yu.

    Impurity iron atoms in vitreous arsenic-selenide As{sub 2}Se{sub 3} films modified by iron form one-electron donor centers with an ionization energy of 0.24 (3) eV (the energy is counted from the conduction-band bottom). The Fermi level is shifted with an increase in the iron concentration from the mid-gap to the donorlevel position of iron due to the filling of one-electron states of the acceptor type lying below the Fermi level. At an iron concentration of ≥3 at %, the electron-exchange process is observed between neutral and ionized iron centers resulting in a change both in the electron density and inmore » the tensor of the electric-field gradient at iron-atom nuclei with increasing temperature above 350 K.« less

  14. Electron shakeoff following the β+ decay of +19Ne and +35Ar trapped ions

    NASA Astrophysics Data System (ADS)

    Fabian, X.; Fléchard, X.; Pons, B.; Liénard, E.; Ban, G.; Breitenfeldt, M.; Couratin, C.; Delahaye, P.; Durand, D.; Finlay, P.; Guillon, B.; Lemière, Y.; Mauger, F.; Méry, A.; Naviliat-Cuncic, O.; Porobic, T.; Quéméner, G.; Severijns, N.; Thomas, J.-C.

    2018-02-01

    The electron shakeoff of 19F and 35Cl atoms resulting from the β+ decay of +19Ne and +35Ar ions has been investigated using a Paul trap coupled to a time of flight recoil-ion spectrometer. The charge-state distributions of the recoiling daughter nuclei were compared to theoretical calculations based on the sudden approximation and accounting for subsequent Auger processes. The excellent agreement obtained for 35Cl is not reproduced in 19F. The shortcoming is attributed to the inaccuracy of the independent particle model employed to calculate the primary shakeoff probabilities in systems with rather low atomic numbers. This calls for more elaborate calculations, including explicitly the electron-electron correlations.

  15. The use of neutron scattering to determine the functional structure of glycoside hydrolase.

    PubMed

    Nakamura, Akihiko; Ishida, Takuya; Samejima, Masahiro; Igarashi, Kiyohiko

    2016-10-01

    Neutron diffraction provides different information from X-ray diffraction, because neutrons are scattered by atomic nuclei, whereas X-rays are scattered by electrons. One of the key advantages of neutron crystallography is the ability to visualize hydrogen and deuterium atoms, making it possible to observe the protonation state of amino acid residues, hydrogen bonds, networks of water molecules and proton relay pathways in enzymes. But, because of technical difficulties, less than 100 enzyme structures have been evaluated by neutron crystallography to date. In this review, we discuss the advantages and disadvantages of neutron crystallography as a tool to investigate the functional structure of glycoside hydrolases, with some examples. Copyright © 2016 Elsevier Ltd. All rights reserved.

  16. Measurements of Reaction Cross Sections for 9-11C

    NASA Astrophysics Data System (ADS)

    Nishizuka, Kenji; Takechi, Maya; Ohtsubo, Takashi; Nishimura, Daiki; Fukuda, Mitsunori; Aoki, Kazuya; Abe, Keijiro; Ikeda, Ayaka; Izumikawa, Takuji; Oikawa, Hiroyuki; Ohnishi, Kosuke; Ohno, Junichi; Ohmika, Shunichiro; Kato, Ikuma; Kanke, Yuki; Kanbe, Shunsuke; Kanda, Naoto; Kikuchi, Haruka; Kitagawa, Atsushi; Sato, Shinji; Sayama, Umito; Shimaya, Jiro; Sugihara, Takanobu; Suzuki, Shinji; Suzuki, Takeshi; Takahashi, Hiroki; Taguchi, Yoshisada; Takei, Yuki; Takeuchi, Yuki; Takenouchi, Arashi; Takemoto, Takanori; Tadano, Natsuki; Tanaka, Masaomi; Tanaka, Yutaro; Chikaato, Kazuya; Du, Hang; Nagai, Takumi; Nagumo, Junya; Fukuda, Shigekazu; Hori, Kensyu; Honma, Akira; Machida, Masahiro; Matsunaga, Satoshi; Mizukami, Atsushi; Mihara, Mototsugu; Miyata, Eri; Murooka, Daiki; Yagi, Shoichi; Yamaoka, Shintaro; Yamaguchi, Takayuki; Yokoyama, Kouhei

    In order to probe the differences of matter and charge radii of atomic nucleus in the proton-rich C isotopes, measurements of reaction cross sections (σR) for 9-11C on proton targets in the energy range from 50 to 120A MeV were performed at HIMAC facility, NIRS. Owing to the large differences between proton-proton and proton-neutron scattering cross sections at this intermediate energy region, σR data for atomic nuclei on proton targets are expected to have the sensitivity to the differences between proton and neutron distributions in the nucleus. Present preliminary data are compared with the Glauber calculation, which suggest the larger enhancements of proton distributions in 9C and 10C compared to 11C.

  17. The strong Bell inequalities: A proposed experimental test

    NASA Technical Reports Server (NTRS)

    Fry, Edward S.

    1994-01-01

    All previous experimental tests of Bell inequalities have required additional assumptions. The strong Bell inequalities (i.e. those requiring no additional assumptions) have never been tested. An experiment has been designed that can, for the first time, provide a definitive test of the strong Bell inequalities. Not only will the detector efficiency loophole be closed; but the locality condition will also be rigorously enforced. The experiment involves producing two Hg-199 atoms by a resonant Raman dissociation of a mercury dimer ((199)Hg2) that is in an electronic and nuclear spin singlet state. Bell inequalities can be tested by measuring angular momentum correlations between the spin one-half nuclei of the two Hg-199 atoms. The method used to make these latter measurements will be described.

  18. Paired and interacting galaxies: Conference summary

    NASA Technical Reports Server (NTRS)

    Norman, Colin A.

    1990-01-01

    The author gives a summary of the conference proceedings. The conference began with the presentation of the basic data sets on pairs, groups, and interacting galaxies with the latter being further discussed with respect to both global properties and properties of the galactic nuclei. Then followed the theory, modelling and interpretation using analytic techniques, simulations and general modelling for spirals and ellipticals, starbursts and active galactic nuclei. Before the conference the author wrote down the three questions concerning pairs, groups and interacting galaxies that he hoped would be answered at the meeting: (1) How do they form, including the role of initial conditions, the importance of subclustering, the evolution of groups to compact groups, and the fate of compact groups; (2) How do they evolve, including issues such as relevant timescales, the role of halos and the problem of overmerging, the triggering and enhancement of star formation and activity in the galactic nuclei, and the relative importance of dwarf versus giant encounters; and (3) Are they important, including the frequency of pairs and interactions, whether merging and interactions are very important aspects of the life of a normal galaxy at formation, during its evolution, in forming bars, shells, rings, bulges, etc., and in the formation and evolution of active galaxies? Where possible he focuses on these three central issues in the summary.

  19. Search for variation of fundamental constants and violations of fundamental symmetries using isotope comparisons

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Berengut, J. C.; Flambaum, V. V.; Kava, E. M.

    2011-10-15

    Atomic microwave clocks based on hyperfine transitions, such as the caesium standard, tick with a frequency that is proportional to the magnetic moment of the nucleus. This magnetic moment varies strongly between isotopes of the same atom, while all atomic electron parameters remain the same. Therefore the comparison of two microwave clocks based on different isotopes of the same atom can be used to constrain variation of fundamental constants. In this paper, we calculate the neutron and proton contributions to the nuclear magnetic moments, as well as their sensitivity to any potential quark-mass variation, in a number of isotopes ofmore » experimental interest including {sup 201,199}Hg and {sup 87,85}Rb, where experiments are underway. We also include a brief treatment of the dependence of the hyperfine transitions to variation in nuclear radius, which in turn is proportional to any change in quark mass. Our calculations of expectation values of proton and neutron spin in nuclei are also needed to interpret measurements of violations of fundamental symmetries.« less

  20. 10 CFR 780.45 - Criteria for decision to issue a license.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... Pursuant to Section 153c of the Atomic Energy Act of 1954 § 780.45 Criteria for decision to issue a license... patent is of primary importance in the production or utilization of special nuclear material or atomic...

  1. 10 CFR 780.45 - Criteria for decision to issue a license.

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... Pursuant to Section 153c of the Atomic Energy Act of 1954 § 780.45 Criteria for decision to issue a license... patent is of primary importance in the production or utilization of special nuclear material or atomic...

  2. 10 CFR 780.45 - Criteria for decision to issue a license.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... Pursuant to Section 153c of the Atomic Energy Act of 1954 § 780.45 Criteria for decision to issue a license... patent is of primary importance in the production or utilization of special nuclear material or atomic...

  3. 10 CFR 780.45 - Criteria for decision to issue a license.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... Pursuant to Section 153c of the Atomic Energy Act of 1954 § 780.45 Criteria for decision to issue a license... patent is of primary importance in the production or utilization of special nuclear material or atomic...

  4. 10 CFR 780.45 - Criteria for decision to issue a license.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... Pursuant to Section 153c of the Atomic Energy Act of 1954 § 780.45 Criteria for decision to issue a license... patent is of primary importance in the production or utilization of special nuclear material or atomic...

  5. DYNAMIC DEUTERIUM ENRICHMENT IN COMETARY WATER VIA ELEY–RIDEAL REACTIONS

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yao, Yunxi; Giapis, Konstantinos P., E-mail: giapis@cheme.caltech.edu

    2017-01-20

    The deuterium-to-hydrogen ratio (D/H) in water found in the coma of Jupiter family comet (JFC) 67P/Churyumov–Gerasimenko was reported to be (5.3 ± 0.7) × 10{sup −4}, the highest among comets and three times the value for other JFCs with an ocean-like ratio. This discrepancy suggests the diverse origins of JFCs and clouds the issue of the origin of Earth’s oceanic water. Here we demonstrate that Eley–Rideal reactions between accelerated water ions and deuterated cometary surface analogs can lead to instantaneous deuterium enrichment in water scattered from the surface. The reaction proceeds with H{sub 2}O{sup +} abstracting adsorbed D atoms, formingmore » an excited H{sub 2}DO* state, which dissociates subsequently to produce energetic HDO. Hydronium ions are also produced readily by the abstraction of H atoms, consistent with H{sub 3}O{sup +} detection and abundance in various comets. Experiments with water isotopologs and kinematic analysis on deuterated platinum surfaces confirmed the dynamic abstraction mechanism. The instantaneous fractionation process is independent of the surface temperature and may operate on the surface of cometary nuclei or dust grains, composed of deuterium-rich silicates and carbonaceous chondrites. The requisite energetic water ions have been detected in the coma of 67P in two populations. This dynamic fractionation process may temporarily increase the water D/H ratio, especially as the comet gets closer to the Sun. The magnitude of the effect depends on the water ion energy-flux and the deuterium content of the exposed cometary surfaces.« less

  6. The compression-mode giant resonances and nuclear incompressibility

    NASA Astrophysics Data System (ADS)

    Garg, Umesh; Colò, Gianluca

    2018-07-01

    The compression-mode giant resonances, namely the isoscalar giant monopole and isoscalar giant dipole modes, are examples of collective nuclear motion. Their main interest stems from the fact that one hopes to extrapolate from their properties the incompressibility of uniform nuclear matter, which is a key parameter of the nuclear Equation of State (EoS). Our understanding of these issues has undergone two major jumps, one in the late 1970s when the Isoscalar Giant Monopole Resonance (ISGMR) was experimentally identified, and another around the turn of the millennium since when theory has been able to start giving reliable error bars to the incompressibility. However, mainly magic nuclei have been involved in the deduction of the incompressibility from the vibrations of finite nuclei. The present review deals with the developments beyond all this. Experimental techniques have been improved, and new open-shell, and deformed, nuclei have been investigated. The associated changes in our understanding of the problem of the nuclear incompressibility are discussed. New theoretical models, decay measurements, and the search for the evolution of compressional modes in exotic nuclei are also discussed.

  7. Self-consistent description of the SHFB equations for 112Sn

    NASA Astrophysics Data System (ADS)

    Ghafouri, M.; Sadeghi, H.; Torkiha, M.

    2018-03-01

    The Hartree-Fock (HF) method is an excellent approximation of the closed shell magic nuclei. Pair correlation is essential for the description of open shell nuclei and has been derived for even-even, odd-odd and even-odd nuclei. These effects are reported by Hartree-Fock with BCS (HFBCS) or Hartree-Fock-Bogolyubov (HFB). These issues have been investigated, especially in the nuclear charts, and such studies have been compared with the observed information. We compute observations such as total binding energy, charge radius, densities, separation energies, pairing gaps and potential energy surfaces for neutrons and protons, and compare them with experimental data and the result of the spherical codes. In spherical even-even neutron-rich nuclei are considered in the Skyrme-Hartree-Fock-Bogolyubov (SHFB) method with density-dependent pairing interaction. Zero-range density-dependent interactions is used in the pairing channel. We solve SHF or SHFB equations in the spatial coordinates with spherical symmetry for tin isotopes such as 112Sn. The numerical accuracy of solving equations in the coordinate space is much greater than the fundamental extensions, which yields almost precise results.

  8. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Thayer, K.J.

    The past year has seen several of the Physics Division`s new research projects reach major milestones with first successful experiments and results: the atomic physics station in the Basic Energy Sciences Research Center at the Argonne Advanced Photon Source was used in first high-energy, high-brilliance x-ray studies in atomic and molecular physics; the Short Orbit Spectrometer in Hall C at the Thomas Jefferson National Accelerator (TJNAF) Facility that the Argonne medium energy nuclear physics group was responsible for, was used extensively in the first round of experiments at TJNAF; at ATLAS, several new beams of radioactive isotopes were developed andmore » used in studies of nuclear physics and nuclear astrophysics; the new ECR ion source at ATLAS was completed and first commissioning tests indicate excellent performance characteristics; Quantum Monte Carlo calculations of mass-8 nuclei were performed for the first time with realistic nucleon-nucleon interactions using state-of-the-art computers, including Argonne`s massively parallel IBM SP. At the same time other future projects are well under way: preparations for the move of Gammasphere to ATLAS in September 1997 have progressed as planned. These new efforts are imbedded in, or flowing from, the vibrant ongoing research program described in some detail in this report: nuclear structure and reactions with heavy ions; measurements of reactions of astrophysical interest; studies of nucleon and sub-nucleon structures using leptonic probes at intermediate and high energies; atomic and molecular structure with high-energy x-rays. The experimental efforts are being complemented with efforts in theory, from QCD to nucleon-meson systems to structure and reactions of nuclei. Finally, the operation of ATLAS as a national users facility has achieved a new milestone, with 5,800 hours beam on target for experiments during the past fiscal year.« less

  9. Parameterization of fission barrier heights of medium, heavy and super heavy nuclei

    NASA Astrophysics Data System (ADS)

    Manjunatha, H. C.

    2017-12-01

    A new semi empirical formula is proposed for fission barrier heights of medium, heavy and super heavy nuclei in the atomic number region 50 ≤ Z ≤ 130. The fitting parameters for the proposed formula are obtained by making a polynomial fit to the available theoretical and experimental data. The calculated fission barrier heights are compared with that of experiments and other theoretical models such as SHF(SLy6) (Burvenich et al. in Phys Rev C 69:014307, 2004), SHFB(SkM) (Baran et al. in Nucl Phys A 944:442, 2015), FRLDM (Möller et al. in Phys Rev C 79:064304, 2009), ETFSI (SkSC4) with Skyrme SkSC4 force (Mamdouh et al. in Nucl Phys A 679:337, 2001), WS (Kowal et al. in Phys Rev C 82:014303, 2010) and CDFT(DD-ME2) (Abusara et al. in Phys Rev C 85:024314, 2012). The standard deviation for fission barrier heights produced by present formula is evaluated. The good agreement of present formula with the experiments and other models suggests that the present formula could be used to evaluate the fission barrier heights of medium, heavy and super heavy nuclei in the region 50 ≤ Z ≤ 130. This formula is a first of its kind that produces fission barrier heights of 2858 nuclei with the only simple inputs of only neutron number (N), proton number (Z) and mass number (A).

  10. Parameterization of fission barrier heights of medium, heavy and super heavy nuclei

    NASA Astrophysics Data System (ADS)

    Manjunatha, H. C.

    2018-04-01

    A new semi empirical formula is proposed for fission barrier heights of medium, heavy and super heavy nuclei in the atomic number region 50 ≤ Z ≤ 130. The fitting parameters for the proposed formula are obtained by making a polynomial fit to the available theoretical and experimental data. The calculated fission barrier heights are compared with that of experiments and other theoretical models such as SHF(SLy6) (Burvenich et al. in Phys Rev C 69:014307, 2004), SHFB(SkM) (Baran et al. in Nucl Phys A 944:442, 2015), FRLDM (Möller et al. in Phys Rev C 79:064304, 2009), ETFSI (SkSC4) with Skyrme SkSC4 force (Mamdouh et al. in Nucl Phys A 679:337, 2001), WS (Kowal et al. in Phys Rev C 82:014303, 2010) and CDFT(DD-ME2) (Abusara et al. in Phys Rev C 85:024314, 2012). The standard deviation for fission barrier heights produced by present formula is evaluated. The good agreement of present formula with the experiments and other models suggests that the present formula could be used to evaluate the fission barrier heights of medium, heavy and super heavy nuclei in the region 50 ≤ Z ≤ 130. This formula is a first of its kind that produces fission barrier heights of 2858 nuclei with the only simple inputs of only neutron number (N), proton number (Z) and mass number (A).

  11. Physical processes in comets

    NASA Technical Reports Server (NTRS)

    Whipple, F. L.; Huebner, W. F.

    1976-01-01

    The paper discusses physical processes in comets which involve solar and nuclear radial forces that affect the motions of gases and icy grains, gas-phase chemistry very close to the nuclei of large comets near the sun, sublimation of icy grains, dissociation of parent molecules into radicals and of radicals into atoms, and ionization by sunlight and collisions. The composition and dimensions of nuclei are examined along with variations in intrinsic brightness, the nature of volatiles, gas production rates in the coma, characteristics of icy grains in the coma, and the structure of streamers, ion tails, and dust tails. The structure of the coma is described in detail on the basis of spectroscopic observations of several comets. The origin of comets is briefly reviewed together with the relation of comets to earth, the interplanetary complex, and the interstellar medium. Desirable future observations are noted, especially by space missions to comets.

  12. The tightly bound nuclei in the liquid drop model

    NASA Astrophysics Data System (ADS)

    Sree Harsha, N. R.

    2018-05-01

    In this paper, we shall maximise the binding energy per nucleon function in the semi-empirical mass formula of the liquid drop model of the atomic nuclei to analytically prove that the mean binding energy per nucleon curve has local extrema at A ≈ 58.6960, Z ≈ 26.3908 and at A ≈ 62.0178, Z ≈ 27.7506. The Lagrange method of multipliers is used to arrive at these results, while we have let the values of A and Z take continuous fractional values. The shell model that shows why 62Ni is the most tightly bound nucleus is outlined. A brief account on stellar nucleosynthesis is presented to show why 56Fe is more abundant than 62Ni and 58Fe. We believe that the analytical proof presented in this paper can be a useful tool to the instructors to introduce the nucleus with the highest mean binding energy per nucleon.

  13. A method to obtain static potential for electron-molecule scattering

    NASA Astrophysics Data System (ADS)

    Srivastava, Rajesh; Das, Tapasi; Stauffer, Allan

    2014-05-01

    Electron scattering from molecules is complicated by the fact that molecules are a multi-centered target with the nuclei of the constituent atoms being a center of charge. One of the most important parts of a scattering calculation is to obtain the static potential which represents the interaction of the incident electron with the unperturbed charge distribution of the molecule. A common way to represent the charge distribution of molecules is with Gaussian orbitals centered on the various nuclei. We have derived a way to calculate spherically-averaged molecular static potentials using this form of molecular wave function which is mostly analytic. This method has been applied to elastic electron scattering from water molecules and we obtained differential cross sections which are compared with previous experimental and theoretical results. The method can be extended to more complex molecules. One of us (RS) is thankful to IAEA, Vienna, Austria and DAE-BRNS, Mumbai, India for financial support.

  14. α decay and cluster radioactivity of nuclei of interest to the synthesis of Z =119 , 120 isotopes

    NASA Astrophysics Data System (ADS)

    Poenaru, D. N.; Gherghescu, R. A.

    2018-04-01

    Super-heavy nuclei of interest for the forthcoming synthesis of the isotopes with Z =119 , 120 are investigated. One of the very interesting latest experiments was performed at the velocity filter SHIP (GSI Darmstadt) trying to produce 299120 in a fusion reaction 248Cm(54Cr,3 n )299120 . We report calculations of α -decay half-lives using four models: AKRA (Akrawy), ASAF (analytical superasymmetric fission), UNIV (universal formula), and semFIS (semi-empirical formula based on fission theory). The released energy, Q , is calculated using the theoretical model of atomic masses, WS4. For Sr,9492 cluster radioactivity of 120,302300 we predict a branching ratio relative to α decay of -0.10 and 0.49, respectively, meaning that it is worth trying to detect such kinds of decay modes in competition with α decay.

  15. Visualizing and Steering Dissociative Frustrated Double Ionization of Hydrogen Molecules

    NASA Astrophysics Data System (ADS)

    Zhang, Wenbin; Yu, Zuqing; Gong, Xiaochun; Wang, Junping; Lu, Peifen; Li, Hui; Song, Qiying; Ji, Qinying; Lin, Kang; Ma, Junyang; Li, Hanxiao; Sun, Fenghao; Qiang, Junjie; Zeng, Heping; He, Feng; Wu, Jian

    2017-12-01

    We experimentally visualize the dissociative frustrated double ionization of hydrogen molecules by using few-cycle laser pulses in a pump-probe scheme, in which process the tunneling ionized electron is recaptured by one of the outgoing nuclei of the breaking molecule. Three internuclear distances are recognized to enhance the dissociative frustrated double ionization of molecules at different instants after the first ionization step. The recapture of the electron can be further steered to one of the outgoing nuclei as desired by using phase-controlled two-color laser pulses. Both the experimental measurements and numerical simulations suggest that the Rydberg atom is favored to emit to the direction of the maximum of the asymmetric optical field. Our results on the one hand intuitively visualize the dissociative frustrated double ionization of molecules, and on the other hand open the possibility to selectively excite the heavy fragment ejected from a molecule.

  16. Theoretical investigation of gas-surface interactions

    NASA Technical Reports Server (NTRS)

    Dyall, Kenneth G.

    1990-01-01

    A Dirac-Hartree-Fock code was developed for polyatomic molecules. The program uses integrals over symmetry-adapted real spherical harmonic Gaussian basis functions generated by a modification of the MOLECULE integrals program. A single Gaussian function is used for the nuclear charge distribution, to ensure proper boundary conditions at the nuclei. The Gaussian primitive functions are chosen to satisfy the kinetic balance condition. However, contracted functions which do not necessarily satisfy this condition may be used. The Fock matrix is constructed in the scalar basis and transformed to a jj-coupled 2-spinor basis before diagonalization. The program was tested against numerical results for atoms with a Gaussian nucleus and diatomic molecules with point nuclei. The energies converge on the numerical values as the basis set size is increased. Full use of molecular symmetry (restricted to D sub 2h and subgroups) is yet to be implemented.

  17. The image of the atomic bomb in Japan before Hiroshima.

    PubMed

    Nakao, Maika

    2009-01-01

    This paper traces the roots of the image of the atomic bomb in Japan by investigating the various discourses on atomic energy and atomic weapons in Japanese literature prior to the bombing of Hiroshima in August 1945. Japan is a country that suffered an atomic attack and, at the same time, one of the countries that was engaged in atomic weapons research during the Second World War. During the war, the discourses on atomic weapons were not limited to the military or scientific communities, but included the general public, thus facilitating the creation of a shared image of the atomic bomb as an ultimate weapon. This paper examines how this image was created. This special issue deals with the comparison among different countries, but the purpose of my paper is to deepen this subject by illustrating the differences within a single country in different periods. This research aims to extend the historical perspective concerning the atomic bomb in Japan, and offers another way of looking at this both historical and contemporary issue.

  18. 77 FR 36298 - In the Matter of Maine Yankee Atomic Power Company; Maine Yankee Atomic Power Station...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-06-18

    ... the Matter of Maine Yankee Atomic Power Company; Maine Yankee Atomic Power Station; Confirmatory Order... Regulatory Commission (NRC or the Commission) issued a Confirmatory Order to Maine Yankee Atomic Power...: (301) 492-3342; Email: [email protected] . I Maine Yankee Atomic Power Company (Maine Yankee or the...

  19. Complexity made simple

    NASA Astrophysics Data System (ADS)

    2010-02-01

    With their passion for analysing the world by breaking it down into ever-smaller pieces, most physicists are "reductionists" at heart. Whether through tradition or instinct, our natural inclination is to reduce matter first to molecules and then to atoms and on to nuclei, nucleons, quarks and beyond. But this approach, while astonishingly successful in terms of understanding the fundamental particles and forces of nature, does not always work. In other words, the whole can often be more than the sum of the parts.

  20. Physics of Spin-Polarized Media

    DTIC Science & Technology

    2007-11-21

    midsection of the cell serving as the cathode, and liquid molten salt outside the cell serving as the anode [5]. This new method is very promising for of...filling atomic clock and magnetometer cells by electrolysis through the glass walls; (6) new investigations of optical pumping and magnetic resonances...cesium vapor can be used to polarize 3 Cs nuclei in CsH salt that coats the walls of a vapor cell. This result, an important first step, has been

  1. Cosmic-ray abundances of the even charge elements from Sn-50 to Ce-58 measured on HEAO-3

    NASA Technical Reports Server (NTRS)

    Stone, E. C.; Garrard, T. L.; Krombel, K. E.; Binns, W. R.; Israel, M. H.; Klarmann, J.; Brewster, N. R.; Fickle, R. K.; Waddington, C. J.

    1983-01-01

    Elements with even atomic number (Z) in the interval Z = 50-58 have been resolved in the cosmic radiation using the Heavy Nuclei Experiment on the HEAO-3 satellite. The observation that Sn-50 and Ba-56 are more abundant than Te-52 and Xe-54 indicates a substantial s-process contribution to the cosmic ray source. A significant abundance of Ce-58 provides further support for this finding.

  2. Complete solution of electronic excitation and ionization in electron-hydrogen molecule scattering

    DOE PAGES

    Zammit, Mark C.; Savage, Jeremy S.; Fursa, Dmitry V.; ...

    2016-06-08

    The convergent close-coupling method has been used to solve the electron-hydrogen molecule scattering problem in the fixed-nuclei approximation. Excellent agreement with experiment is found for the grand total, elastic, electronic-excitation, and total ionization cross sections from the very low to the very high energies. This shows that for the electronic degrees of freedom the method provides a complete treatment of electron scattering on molecules as it does for atoms.

  3. Neutron production by cosmic-ray muons in various materials

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Manukovsky, K. V.; Ryazhskaya, O. G.; Sobolevsky, N. M.

    The results obtained by studying the background of neutrons produced by cosmic-raymuons in underground experimental facilities intended for rare-event searches and in surrounding rock are presented. The types of this rock may include granite, sedimentary rock, gypsum, and rock salt. Neutron production and transfer were simulated using the Geant4 and SHIELD transport codes. These codes were tuned via a comparison of the results of calculations with experimental data—in particular, with data of the Artemovsk research station of the Institute for Nuclear Research (INR, Moscow, Russia)—as well as via an intercomparison of results of calculations with the Geant4 and SHIELD codes.more » It turns out that the atomic-number dependence of the production and yield of neutrons has an irregular character and does not allow a description in terms of a universal function of the atomic number. The parameters of this dependence are different for two groups of nuclei—nuclei consisting of alpha particles and all of the remaining nuclei. Moreover, there are manifest exceptions from a power-law dependence—for example, argon. This may entail important consequences both for the existing underground experimental facilities and for those under construction. Investigation of cosmic-ray-induced neutron production in various materials is of paramount importance for the interpretation of experiments conducted at large depths under the Earth’s surface.« less

  4. Practical Applications of Cosmic Ray Science: Spacecraft, Aircraft, Ground-Based Computation and Control Systems, Exploration, and Human Health and Safety

    NASA Technical Reports Server (NTRS)

    Koontz, Steve

    2015-01-01

    In this presentation a review of galactic cosmic ray (GCR) effects on microelectronic systems and human health and safety is given. The methods used to evaluate and mitigate unwanted cosmic ray effects in ground-based, atmospheric flight, and space flight environments are also reviewed. However not all GCR effects are undesirable. We will also briefly review how observation and analysis of GCR interactions with planetary atmospheres and surfaces and reveal important compositional and geophysical data on earth and elsewhere. About 1000 GCR particles enter every square meter of Earth’s upper atmosphere every second, roughly the same number striking every square meter of the International Space Station (ISS) and every other low- Earth orbit spacecraft. GCR particles are high energy ionized atomic nuclei (90% protons, 9% alpha particles, 1% heavier nuclei) traveling very close to the speed of light. The GCR particle flux is even higher in interplanetary space because the geomagnetic field provides some limited magnetic shielding. Collisions of GCR particles with atomic nuclei in planetary atmospheres and/or regolith as well as spacecraft materials produce nuclear reactions and energetic/highly penetrating secondary particle showers. Three twentieth century technology developments have driven an ongoing evolution of basic cosmic ray science into a set of practical engineering tools needed to design, test, and verify the safety and reliability of modern complex technological systems and assess effects on human health and safety effects. The key technology developments are: 1) high altitude commercial and military aircraft; 2) manned and unmanned spacecraft; and 3) increasingly complex and sensitive solid state micro-electronics systems. Space and geophysical exploration needs drove the development of the instruments and analytical tools needed to recover compositional and structural data from GCR induced nuclear reactions and secondary particle showers. Finally, the possible role of GCR secondary particle showers in addressing an important homeland security problem, finding nuclear contraband and weapons, will be briefly reviewed.

  5. Precision muon physics

    NASA Astrophysics Data System (ADS)

    Gorringe, T. P.; Hertzog, D. W.

    2015-09-01

    The muon is playing a unique role in sub-atomic physics. Studies of muon decay both determine the overall strength and establish the chiral structure of weak interactions, as well as setting extraordinary limits on charged-lepton-flavor-violating processes. Measurements of the muon's anomalous magnetic moment offer singular sensitivity to the completeness of the standard model and the predictions of many speculative theories. Spectroscopy of muonium and muonic atoms gives unmatched determinations of fundamental quantities including the magnetic moment ratio μμ /μp, lepton mass ratio mμ /me, and proton charge radius rp. Also, muon capture experiments are exploring elusive features of weak interactions involving nucleons and nuclei. We will review the experimental landscape of contemporary high-precision and high-sensitivity experiments with muons. One focus is the novel methods and ingenious techniques that achieve such precision and sensitivity in recent, present, and planned experiments. Another focus is the uncommonly broad and topical range of questions in atomic, nuclear and particle physics that such experiments explore.

  6. A simple scaling law for the equation of state and the radial distribution functions calculated by density-functional theory molecular dynamics

    NASA Astrophysics Data System (ADS)

    Danel, J.-F.; Kazandjian, L.

    2018-06-01

    It is shown that the equation of state (EOS) and the radial distribution functions obtained by density-functional theory molecular dynamics (DFT-MD) obey a simple scaling law. At given temperature, the thermodynamic properties and the radial distribution functions given by a DFT-MD simulation remain unchanged if the mole fractions of nuclei of given charge and the average volume per atom remain unchanged. A practical interest of this scaling law is to obtain an EOS table for a fluid from that already obtained for another fluid if it has the right characteristics. Another practical interest of this result is that an asymmetric mixture made up of light and heavy atoms requiring very different time steps can be replaced by a mixture of atoms of equal mass, which facilitates the exploration of the configuration space in a DFT-MD simulation. The scaling law is illustrated by numerical results.

  7. Electronic torsional sound in linear atomic chains: Chemical energy transport at 1000 km/s

    NASA Astrophysics Data System (ADS)

    Kurnosov, Arkady A.; Rubtsov, Igor V.; Maksymov, Andrii O.; Burin, Alexander L.

    2016-07-01

    We investigate entirely electronic torsional vibrational modes in linear cumulene chains. The carbon nuclei of a cumulene are positioned along the primary axis so that they can participate only in the transverse and longitudinal motions. However, the interatomic electronic clouds behave as a torsion spring with remarkable torsional stiffness. The collective dynamics of these clouds can be described in terms of electronic vibrational quanta, which we name torsitons. It is shown that the group velocity of the wavepacket of torsitons is much higher than the typical speed of sound, because of the small mass of participating electrons compared to the atomic mass. For the same reason, the maximum energy of the torsitons in cumulenes is as high as a few electronvolts, while the minimum possible energy is evaluated as a few hundred wavenumbers and this minimum is associated with asymmetry of zero point atomic vibrations. Theory predictions are consistent with the time-dependent density functional theory calculations. Molecular systems for experimental evaluation of the predictions are proposed.

  8. Neutron Nucleic Acid Crystallography.

    PubMed

    Chatake, Toshiyuki

    2016-01-01

    The hydration shells surrounding nucleic acids and hydrogen-bonding networks involving water molecules and nucleic acids are essential interactions for the structural stability and function of nucleic acids. Water molecules in the hydration shells influence various conformations of DNA and RNA by specific hydrogen-bonding networks, which often contribute to the chemical reactivity and molecular recognition of nucleic acids. However, X-ray crystallography could not provide a complete description of structural information with respect to hydrogen bonds. Indeed, X-ray crystallography is a powerful tool for determining the locations of water molecules, i.e., the location of the oxygen atom of H2O; however, it is very difficult to determine the orientation of the water molecules, i.e., the orientation of the two hydrogen atoms of H2O, because X-ray scattering from the hydrogen atom is very small.Neutron crystallography is a specialized tool for determining the positions of hydrogen atoms. Neutrons are not diffracted by electrons, but are diffracted by atomic nuclei; accordingly, neutron scattering lengths of hydrogen and its isotopes are comparable to those of non-hydrogen atoms. Therefore, neutron crystallography can determine both of the locations and orientations of water molecules. This chapter describes the current status of neutron nucleic acid crystallographic research as well as the basic principles of neutron diffraction experiments performed on nucleic acid crystals: materials, crystallization, diffraction experiments, and structure determination.

  9. Atomic force microscopy study on crystal growth of Cu 2+-doped L-arginine phosphate monohydrate crystals

    NASA Astrophysics Data System (ADS)

    Geng, Y. L.; Xu, D.; Wang, Y. L.; Du, W.; Liu, H. Y.; Zhang, G. H.; Wang, X. Q.; Sun, D. L.

    2005-01-01

    Sub-steps and defects of the {1 0 0} planes of Cu 2+-doped L-arginine phosphate monohydrate (LAP) crystals are observed by atomic force microscopy. Formation of sub-steps is not due to the stacking faults but a result of single LAP: Cu 2+ molecule acting as growth unit. Two-dimensional (2D) nuclei with the same height as sub-steps occur on the step-edges. Impurities of Cu 2+ ions cause steps bunch and macrosteps formation. Liquid inclusions in the form of long channels form when the macrosteps lose their stability. Numerous small 3D growth hillocks are found in the channels. The extra stress induced by the 3D islands can result in dislocations and steps mismatches.

  10. Scissors Mode of Dipolar Quantum Droplets of Dysprosium Atoms

    NASA Astrophysics Data System (ADS)

    Ferrier-Barbut, Igor; Wenzel, Matthias; Böttcher, Fabian; Langen, Tim; Isoard, Mathieu; Stringari, Sandro; Pfau, Tilman

    2018-04-01

    We report on the observation of the scissors mode of a single dipolar quantum droplet. The existence of this mode is due to the breaking of the rotational symmetry by the dipole-dipole interaction, which is fixed along an external homogeneous magnetic field. By modulating the orientation of this magnetic field, we introduce a new spectroscopic technique for studying dipolar quantum droplets. This provides a precise probe for interactions in the system, allowing us to extract a background scattering length for 164Dy of 69 (4 )a0 . Our results establish an analogy between quantum droplets and atomic nuclei, where the existence of the scissors mode is also only due to internal interactions. They further open the possibility to explore physics beyond the available theoretical models for strongly dipolar quantum gases.

  11. Observation of three-photon bound states in a quantum nonlinear medium

    NASA Astrophysics Data System (ADS)

    Liang, Qi-Yu; Venkatramani, Aditya V.; Cantu, Sergio H.; Nicholson, Travis L.; Gullans, Michael J.; Gorshkov, Alexey V.; Thompson, Jeff D.; Chin, Cheng; Lukin, Mikhail D.; Vuletić, Vladan

    2018-02-01

    Bound states of massive particles, such as nuclei, atoms, or molecules, constitute the bulk of the visible world around us. By contrast, photons typically only interact weakly. We report the observation of traveling three-photon bound states in a quantum nonlinear medium where the interactions between photons are mediated by atomic Rydberg states. Photon correlation and conditional phase measurements reveal the distinct bunching and phase features associated with three-photon and two-photon bound states. Such photonic trimers and dimers possess shape-preserving wave functions that depend on the constituent photon number. The observed bunching and strongly nonlinear optical phase are described by an effective field theory of Rydberg-induced photon-photon interactions. These observations demonstrate the ability to realize and control strongly interacting quantum many-body states of light.

  12. Applications of Quantum Theory of Atomic and Molecular Scattering to Problems in Hypersonic Flow

    NASA Technical Reports Server (NTRS)

    Malik, F. Bary

    1995-01-01

    The general status of a grant to investigate the applications of quantum theory in atomic and molecular scattering problems in hypersonic flow is summarized. Abstracts of five articles and eleven full-length articles published or submitted for publication are included as attachments. The following topics are addressed in these articles: fragmentation of heavy ions (HZE particles); parameterization of absorption cross sections; light ion transport; emission of light fragments as an indicator of equilibrated populations; quantum mechanical, optical model methods for calculating cross sections for particle fragmentation by hydrogen; evaluation of NUCFRG2, the semi-empirical nuclear fragmentation database; investigation of the single- and double-ionization of He by proton and anti-proton collisions; Bose-Einstein condensation of nuclei; and a liquid drop model in HZE particle fragmentation by hydrogen.

  13. Volume 10, Issue 11-12© 2001 WILEY-VCH Verlag Berlin GmbH, Fed. Rep. of GermanySave Title to My Profile

    E-MailPrint

    Volume 10, Issue 11-12, Pages 887-984(November 2001)

    Original Paper

    Imaging of atomic orbitals with the Atomic Force Microscope - experiments and simulations

    NASA Astrophysics Data System (ADS)

    Giessibl, F. J.; Bielefeldt, H.; Hembacher, S.; Mannhart, J.

    2001-11-01

    Atomic force microscopy (AFM) is a mechanical profiling technique that allows to image surfaces with atomic resolution. Recent progress in reducing the noise of this technique has led to a resolution level where previously undetectable symmetries of the images of single atoms are observed. These symmetries are related to the nature of the interatomic forces. The Si(111)-(7 × 7) surface is studied by AFM with various tips and AFM images are simulated with chemical and electrostatic model forces. The calculation of images from the tip-sample forces is explained in detail and the implications of the imaging parameters are discussed. Because the structure of the Si(111)-(7 × 7) surface is known very well, the shape of the adatom images is used to determine the tip structure. The observability of atomic orbitals by AFM and scanning tunneling microscopy is discussed.

  14. Self-bound droplets of a dilute magnetic quantum liquid

    NASA Astrophysics Data System (ADS)

    Schmitt, Matthias; Wenzel, Matthias; Böttcher, Fabian; Ferrier-Barbut, Igor; Pfau, Tilman

    2016-11-01

    Self-bound many-body systems are formed through a balance of attractive and repulsive forces and occur in many physical scenarios. Liquid droplets are an example of a self-bound system, formed by a balance of the mutual attractive and repulsive forces that derive from different components of the inter-particle potential. It has been suggested that self-bound ensembles of ultracold atoms should exist for atom number densities that are 108 times lower than in a helium droplet, which is formed from a dense quantum liquid. However, such ensembles have been elusive up to now because they require forces other than the usual zero-range contact interaction, which is either attractive or repulsive but never both. On the basis of the recent finding that an unstable bosonic dipolar gas can be stabilized by a repulsive many-body term, it was predicted that three-dimensional self-bound quantum droplets of magnetic atoms should exist. Here we report the observation of such droplets in a trap-free levitation field. We find that this dilute magnetic quantum liquid requires a minimum, critical number of atoms, below which the liquid evaporates into an expanding gas as a result of the quantum pressure of the individual constituents. Consequently, around this critical atom number we observe an interaction-driven phase transition between a gas and a self-bound liquid in the quantum degenerate regime with ultracold atoms. These droplets are the dilute counterpart of strongly correlated self-bound systems such as atomic nuclei and helium droplets.

  15. Self-bound droplets of a dilute magnetic quantum liquid.

    PubMed

    Schmitt, Matthias; Wenzel, Matthias; Böttcher, Fabian; Ferrier-Barbut, Igor; Pfau, Tilman

    2016-11-10

    Self-bound many-body systems are formed through a balance of attractive and repulsive forces and occur in many physical scenarios. Liquid droplets are an example of a self-bound system, formed by a balance of the mutual attractive and repulsive forces that derive from different components of the inter-particle potential. It has been suggested that self-bound ensembles of ultracold atoms should exist for atom number densities that are 10 8 times lower than in a helium droplet, which is formed from a dense quantum liquid. However, such ensembles have been elusive up to now because they require forces other than the usual zero-range contact interaction, which is either attractive or repulsive but never both. On the basis of the recent finding that an unstable bosonic dipolar gas can be stabilized by a repulsive many-body term, it was predicted that three-dimensional self-bound quantum droplets of magnetic atoms should exist. Here we report the observation of such droplets in a trap-free levitation field. We find that this dilute magnetic quantum liquid requires a minimum, critical number of atoms, below which the liquid evaporates into an expanding gas as a result of the quantum pressure of the individual constituents. Consequently, around this critical atom number we observe an interaction-driven phase transition between a gas and a self-bound liquid in the quantum degenerate regime with ultracold atoms. These droplets are the dilute counterpart of strongly correlated self-bound systems such as atomic nuclei and helium droplets.

  16. Induced starburst and nuclear activity: Faith, facts, and theory

    NASA Technical Reports Server (NTRS)

    Shlosman, Isaac

    1990-01-01

    The problem of the origin of starburst and nuclear (nonstellar) activity in galaxies is reviewed. A physical understanding of the mechanism(s) that induce both types of activity requires one to address the following issues: (1) what is the source of fuel that powers starbursts and active galactic nuclei; and (2) how is it channeled towards the central regions of host galaxies? As a possible clue, the author examines the role of non-axisymmetric perturbations of galactic disks and analyzes their potential triggers. Global gravitational instabilities in the gas on scales approx. 100 pc appear to be crucial for fueling the active galactic nuclei.

  17. Atomic cluster collisions

    NASA Astrophysics Data System (ADS)

    Korol, Andrey V.; Solov'yov, Andrey

    2013-01-01

    Atomic cluster collisions are a field of rapidly emerging research interest by both experimentalists and theorists. The international symposium on atomic cluster collisions (ISSAC) is the premier forum to present cutting-edge research in this field. It was established in 2003 and the most recent conference was held in Berlin, Germany in July of 2011. This Topical Issue presents original research results from some of the participants, who attended this conference. This issues specifically focuses on two research areas, namely Clusters and Fullerenes in External Fields and Nanoscale Insights in Radiation Biodamage.

  18. Hydrothermal Crystal Growth of Lithium Tetraborate and Lithium Gamma-Metaborate

    DTIC Science & Technology

    2014-03-27

    could be atomic nuclei, the center of mass of some complex—those details are immaterial. Both the rectangle and lozenge form potential cross-sections...HR y d L Figure 10. The red lines are the various contours of solution of 9, using a = 10 Bohr radii and the mass of coefficients on the LHS forced to...absorptivity is significantly below that of the transition metals or the actinides [9]. The lithium borate crystals are therefore a strong candidate for

  19. LEAP 1992: Conference summary

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dover, C.B.

    1992-12-01

    We present a summary of the many new results in antiproton ({bar p}) physics presented at the LEAP `92 conference, in the areas of meson spectroscopy, {bar N}N scattering, annihilation and spin observables, strangeness and charm production, {bar N} annihilation in nuclei, atomic physics with very low energy {bar p}`s, the exploration of fundamental symmetries and interactions with {bar p} (CP, T, CPT, gravitation), and the prospects for new {bar p} facilities at ultralow energies or energies above the LEAR regime ({ge} 2 GeV/c).

  20. LEAP 1992: Conference summary

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dover, C.B.

    1992-12-01

    We present a summary of the many new results in antiproton ([bar p]) physics presented at the LEAP '92 conference, in the areas of meson spectroscopy, [bar N]N scattering, annihilation and spin observables, strangeness and charm production, [bar N] annihilation in nuclei, atomic physics with very low energy [bar p]'s, the exploration of fundamental symmetries and interactions with [bar p] (CP, T, CPT, gravitation), and the prospects for new [bar p] facilities at ultralow energies or energies above the LEAR regime ([ge] 2 GeV/c).

  1. Towards a Unified Description of the Electroweak Nuclear Response

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Benhar, Omar; Lovato, Alessandro

    2015-06-01

    We briefly review the growing efforts to set up a unified framework for the description of neutrino interactions with atomic nuclei and nuclear matter, applicable in the broad kinematical region corresponding to neutrino energies ranging between few MeV and few GeV. The emerging picture suggests that the formalism of nuclear many-body theory (NMBT) can be exploited to obtain the neutrino-nucleus cross-sections needed for both the interpretation of oscillation signals and simulations of neutrino transport in compact stars

  2. Positronium formation in e+ plus H- collisions

    NASA Technical Reports Server (NTRS)

    Straton, Jack C.; Drachman, Richard J.

    1990-01-01

    Cross sections for positronium formation by capture from the negative hydrogen ion are given. Orthogonalization corrections to the Coulomb (First) Born Approximation (CBA) differential and total cross sections are calculated using approximate H- wave functions of both Lowdin and Chandrasekhar. Various methods of orthogonalizing the unbound projectile to the possible bound states are considered. It is found that treating the atomic nuclei as if they were isotopic spin projections of a single type of nucleon gives cross sections that are an improvement over the CBA.

  3. Correlation of nonorthogonality of best hybrid bond orbitals with bond strength of orthogonal orbitals

    PubMed Central

    Pauling, Linus

    1976-01-01

    An expression is derived for the bond length of two spd orbitals with maximum values in two directions forming a given bond angle by consideration of the nonorthogonality integral of two best orbitals in these directions. This equation is equivalent to the expression derived by formulating the pair of orthogonal orbitals. Similar expressions are derived for spdf orbitals. Applications are made to icosahedral and cuboctahedral bonds and to the packing of nucleons in atomic nuclei. PMID:16578736

  4. Correlation of nonorthogonality of best hybrid bond orbitals with bond strength of orthogonal orbitals.

    PubMed

    Pauling, L

    1976-02-01

    An expression is derived for the bond length of two spd orbitals with maximum values in two directions forming a given bond angle by consideration of the nonorthogonality integral of two best orbitals in these directions. This equation is equivalent to the expression derived by formulating the pair of orthogonal orbitals. Similar expressions are derived for spdf orbitals. Applications are made to icosahedral and cuboctahedral bonds and to the packing of nucleons in atomic nuclei.

  5. Simulation of dependence of the cross section of deuterons beam fragmentation into cumulative pions and protons on the mass of the target nucleus

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Litvinenko, A. G., E-mail: alitvin@jinr.ru; Litvinenko, E. I.

    2015-03-15

    We have studied the mechanisms influencing production of cumulative pions and protons in the fragmentation of the incident deuterons into cumulative pions and protons emitted at zero angle. We argue that the peripheral dependence on the atomic mass of the target nucleus, which was obtained in the experiments for medium and heavy nuclei, can be explained by scattering on target nucleons without introducing additional parameters.

  6. Nuclear physics from lattice QCD at strong coupling.

    PubMed

    de Forcrand, Ph; Fromm, M

    2010-03-19

    We study numerically the strong coupling limit of lattice QCD with one flavor of massless staggered quarks. We determine the complete phase diagram as a function of temperature and chemical potential, including a tricritical point. We clarify the nature of the low temperature dense phase, which is strongly bound "nuclear" matter. This strong binding is explained by the nuclear potential, which we measure. Finally, we determine, from this first-principles limiting case of QCD, the masses of "atomic nuclei" up to A=12 "carbon".

  7. Influence of target thickness on the release of radioactive atoms

    NASA Astrophysics Data System (ADS)

    Guillot, Julien; Roussière, Brigitte; Tusseau-Nenez, Sandrine; Barré-Boscher, Nicole; Borg, Elie; Martin, Julien

    2017-03-01

    Nowadays, intense exotic beams are needed in order to study nuclei with very short half-life. To increase the release efficiency of the fission products, all the target characteristics involved must be improved (e.g. chemical composition, dimensions, physicochemical properties such as grain size, porosity, density…). In this article, we study the impact of the target thickness. Released fractions measured from graphite and uranium carbide pellets are presented as well as Monte-Carlo simulations of the Brownian motion.

  8. Masses from an inhomogeneous partial difference equation with higher-order isospin contributions

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Masson, P.J.; Jaenecke, J.

    In the present work, a mass equation obtained as the solution of an inhomogeneous partial difference equation is used to predict masses of unknown neutron-rich and proton-rich nuclei. The inhomogeneous source terms contain shell-dependent symmetry energy expressions (quadratic in isospin), and include, as well, an independently derived shell-model Coulomb energy equation which describes all known Coulomb displacement energies with a standarad deviation of sigma/sub c/ = 41 keV. Perturbations of higher order in isospin, previously recognized as a cause of systematic effects in long-range mass extrapolations, are also incorporated. The most general solutions of the inhomogeneous difference equation have beenmore » deduced from a chi/sup 2/-minimization procedure based on the recent atomic mass adjustment of Wapstra, Audi, and Hoekstra. Subjecting the solutions further to the condition of charge symmetry preserves the accuracy of Coulomb energies and allows mass predictions for nuclei with both Ngreater than or equal toZ and Z>N. The solutions correspond to a mass equation with 470 parameters. Using this equation, 4385 mass values have been calculated for nuclei with Agreater than or equal to16 (except N = Z = odd for A<40), with a standard deviation of sigma/sub m/ = 194 keV from the experimental masses. copyright 1988 Academic Press, Inc.« less

  9. Experimental results on antiproton-nuclei annihilation cross section at very low energies

    NASA Astrophysics Data System (ADS)

    Aghai-Khozani, H.; Barna, D.; Corradini, M.; Hayano, R.; Hori, M.; Kobayashi, T.; Leali, M.; Lodi-Rizzini, E.; Mascagna, V.; Prest, M.; Soter, A.; Todoroki, K.; Vallazza, E.; Venturelli, L.; Zurlo, N.

    2014-03-01

    Investigating the antiproton cross section on nuclei at low energies (1 eV - 1 MeV) is of great interest for fundamental cosmology and nuclear physics as well. The process is of great relevance for the models which try to explain the matter/antimatter asymmetry in the universe assuming the existence of the so-called "island" where antinucleon-nucleon annihilations occur in the border region [1]. For the nuclear physics point of view, the annihilation process is considered a useful tool to evaluate the neutron/proton ratio probing the external region of the nucleus. Moreover, the cross section measured at LEAR in the 80s-90s showed an unexpected behaviour for energies below 1 MeV. The results showed a saturation with the atomic mass number against the A2/3 trend which is known for higher energies. The ASACUSA collaboration at CERN measured 5.3 MeV antiproton annihilation cross section on different nuclei whose results demonstrated to be consistent with the black-disk model with the Coulomb correction [2]. So far, experimental limits prevented the data acquisition for energies below 1 MeV. In 2012 the 100 keV region has been investigated for the first time [3]. We present here the results of the experiment.

  10. Accelerated path integral methods for atomistic simulations at ultra-low temperatures

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Uhl, Felix, E-mail: felix.uhl@rub.de; Marx, Dominik; Ceriotti, Michele

    2016-08-07

    Path integral methods provide a rigorous and systematically convergent framework to include the quantum mechanical nature of atomic nuclei in the evaluation of the equilibrium properties of molecules, liquids, or solids at finite temperature. Such nuclear quantum effects are often significant for light nuclei already at room temperature, but become crucial at cryogenic temperatures such as those provided by superfluid helium as a solvent. Unfortunately, the cost of converged path integral simulations increases significantly upon lowering the temperature so that the computational burden of simulating matter at the typical superfluid helium temperatures becomes prohibitive. Here we investigate how accelerated pathmore » integral techniques based on colored noise generalized Langevin equations, in particular the so-called path integral generalized Langevin equation thermostat (PIGLET) variant, perform in this extreme quantum regime using as an example the quasi-rigid methane molecule and its highly fluxional protonated cousin, CH{sub 5}{sup +}. We show that the PIGLET technique gives a speedup of two orders of magnitude in the evaluation of structural observables and quantum kinetic energy at ultralow temperatures. Moreover, we computed the spatial spread of the quantum nuclei in CH{sub 4} to illustrate the limits of using such colored noise thermostats close to the many body quantum ground state.« less

  11. Extracting nuclear sizes of medium to heavy nuclei from total reaction cross sections

    NASA Astrophysics Data System (ADS)

    Horiuchi, W.; Hatakeyama, S.; Ebata, S.; Suzuki, Y.

    2016-04-01

    Background: Proton and neutron radii are fundamental quantities of atomic nuclei. To study the sizes of short-lived unstable nuclei, there is a need for an alternative to electron scattering. Purpose: The recent paper by Horiuchi et al. [Phys. Rev. C 89, 011601(R) (2014)], 10.1103/PhysRevC.89.011601 proposed a possible way of extracting the matter and neutron-skin thickness of light- to medium-mass nuclei using total reaction cross section, σR. The analysis is extended to medium to heavy nuclei up to lead isotopes with due attention to Coulomb breakup contributions as well as density distributions improved by paring correlation. Methods: We formulate a quantitative calculation of σR based on the Glauber model including the Coulomb breakup. To substantiate the treatment of the Coulomb breakup, we also evaluate the Coulomb breakup cross section due to the electric dipole field in a canonical-basis-time-dependent-Hartree-Fock-Bogoliubov theory in the three-dimensional coordinate space. Results: We analyze σR's of 103 nuclei with Z =20 , 28, 40, 50, 70, and 82 incident on light targets, H,21, 4He, and 12C. Three kinds of Skyrme interactions are tested to generate those wave functions. To discuss possible uncertainty due to the Coulomb breakup, we examine its dependence on the target, the incident energy, and the Skyrme interaction. The proton is a most promising target for extracting the nuclear sizes as the Coulomb excitation can safely be neglected. We find that the so-called reaction radius, aR=√{σR/π } , for the proton target is very well approximated by a linear function of two variables, the matter radius and the skin thickness, in which three constants depend only on the incident energy. We quantify the accuracy of σR measurements needed to extract the nuclear sizes. Conclusions: The proton is the best target because, once the incident energy is set, its aR is very accurately determined by only the matter radius and neutron-skin thickness. If σR's at different incident energies are measured, one can determine both the proton and neutron radii for unstable nuclei as well. The total reaction cross sections calculated in this paper are given as Supplemental Material for the sake of future measurements.

  12. Development of a Plutonium Ceramic Target for the MASHA Separator

    NASA Astrophysics Data System (ADS)

    Shaughnessy, D. A.; Moody, K. J.; Kenneally, J. M.; Wild, J. F.; Stoyer, M. A.; Lougheed, R. W.; Yeremin, A. V.; Oganessian, Yu. Ts.

    2004-04-01

    We are participating in the development of the target for the MASHA (Mass Analyzer of Super Heavy Atoms) on-line mass separator in Dubna. Along with recent upgrades of the U400 cyclotron, MASHA will provide for at least a ten-fold increase in the production- and-detection rate for element 114 atoms, and will allow us to measure their atomic masses precisely. The MASHA separator will employ a thick Pu ceramic target capa- ble of tolerating temperatures in the vicinity of 2000 C without vaporizing the actinide compound. Reaction products will diffuse out of the target and will drift to an ECR ion source after which they will be transported through the separator and will impinge on a position-sensitive focal-plane detector array. Furthermore, operation of the MASHA hot target/ion source combination will provide chemical volatility information that will support our assignment of an atomic number of 114 to these nuclei. Taken together, these experiments on MASHA will allow us to make measurements that will cement our identification of element 114 and provide for future experiments in which the chemical properties of the heaviest elements are studied.

  13. Magnetizabilities of relativistic hydrogenlike atoms in some arbitrary discrete energy eigenstates

    NASA Astrophysics Data System (ADS)

    Stefańska, Patrycja

    2016-03-01

    We present the results of numerical calculations of magnetizability (χ) of the relativistic one-electron atoms with a pointlike, spinless and motionless nuclei of charge Ze. Exploiting the analytical formula for χ recently derived by us Stefańska (2015), valid for an arbitrary discrete energy eigenstate, we have found the values of the magnetizability for the ground state and for the first and the second set of excited states (i.e.: 2s1/2, 2p1/2, 2p3/2, 3s1/2, 3p1/2, 3p3/2, 3d3/2, and 3d5/2) of the Dirac one-electron atom. The results for ions with the atomic number 1 ⩽ Z ⩽ 137 are given in 14 tables. The comparison of the numerical values of magnetizabilities for the ground state and for each state belonging to the first set of excited states of selected hydrogenlike ions, obtained with the use of two different values of the fine-structure constant, i.e.: α-1 = 137.035 999 139 (CODATA 2014) and α-1 = 137.035 999 074 (CODATA 2010), is also presented.

  14. Fast Atom Ionization in Strong Electromagnetic Radiation

    NASA Astrophysics Data System (ADS)

    Apostol, M.

    2018-05-01

    The Goeppert-Mayer and Kramers-Henneberger transformations are examined for bound charges placed in electromagnetic radiation in the non-relativistic approximation. The consistent inclusion of the interaction with the radiation field provides the time evolution of the wavefunction with both structural interaction (which ensures the bound state) and electromagnetic interaction. It is shown that in a short time after switching on the high-intensity radiation the bound charges are set free. In these conditions, a statistical criterion is used to estimate the rate of atom ionization. The results correspond to a sudden application of the electromagnetic interaction, in contrast with the well-known ionization probability obtained by quasi-classical tunneling through classically unavailable non-stationary states, or other equivalent methods, where the interaction is introduced adiabatically. For low-intensity radiation the charges oscillate and emit higher-order harmonics, the charge configuration is re-arranged and the process is resumed. Tunneling ionization may appear in these circumstances. Extension of the approach to other applications involving radiation-induced charge emission from bound states is discussed, like ionization of molecules, atomic clusters or proton emission from atomic nuclei. Also, results for a static electric field are included.

  15. Environmental Durability Issues for Solar Power Systems in Low Earth Orbit

    NASA Technical Reports Server (NTRS)

    Degroh, Kim K.; Banks, Bruce A.; Smith, Daniela C.

    1994-01-01

    Space solar power systems for use in the low Earth orbit (LEO) environment experience a variety of harsh environmental conditions. Materials used for solar power generation in LEO need to be durable to environmental threats such as atomic oxygen, ultraviolet (UV) radiation, thermal cycling, and micrometeoroid and debris impact. Another threat to LEO solar power performance is due to contamination from other spacecraft components. This paper gives an overview of these LEO environmental issues as they relate to space solar power system materials. Issues addressed include atomic oxygen erosion of organic materials, atomic oxygen undercutting of protective coatings, UV darkening of ceramics, UV embrittlement of Teflon, effects of thermal cycling on organic composites, and contamination due to silicone and organic materials. Specific examples of samples from the Long Duration Exposure Facility (LDEF) and materials returned from the first servicing mission of the Hubble Space Telescope (HST) are presented. Issues concerning ground laboratory facilities which simulate the LEO environment are discussed along with ground-to-space correlation issues.

  16. 77 FR 36300 - In the Matter of Connecticut Yankee Atomic Power Company; Haddam Neck Plant; Confirmatory Order...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-06-18

    ... the Matter of Connecticut Yankee Atomic Power Company; Haddam Neck Plant; Confirmatory Order Modifying... Commission (NRC or the Commission) issued a Confirmatory Order to Connecticut Yankee Atomic Power Company...: (301) 492-3342; Email: [email protected] . I Connecticut Yankee Atomic Power Company (Connecticut...

  17. ToF diagnostic of Tin resonant laser photoionization in SPES laser offline laboratory

    NASA Astrophysics Data System (ADS)

    Scarpa, D.; Fedorov, D.; Andrighetto, A.; Mariotti, E.; Nicolosi, P.; Sottili, L.; Tomaselli, A.; Cecchi, R.; Stiaccini, L.

    2016-09-01

    Tin is the principal element of interest in the SPES ISOL facility, which is under construction at Legnaro INFN Laboratories. Atomic nuclei have a shell structure in which nuclei with \\textquoteleft magic numbers\\textquoteright of protons and neutrons are analogous to the noble gasses in atomic physics. In particular, recent theoretical studies, reveal double-magic nature of radioactive 132Sn. For this reason the nuclear physics community demonstrated, in the last years, a huge interest to produce and study this radioactive neutron rich isotope. Experiments on Tin laser resonant ionization have been performed in the offline SPES laser laboratory to investigate the capability of the new home-made Time of Flight (ToF) mass spectrometer. Several three-step, two color ionization schemes have been tested by comparing fast and slow optogalvanic signals from a Tin Hollow Cathode Lamp (HCL) and Time of Flight signals from the spectrometer. By scanning the wavelength of one of the two dye lasers across the specific resonance, comparisons of ionization signals from both the ToF and the HCL have been made, finding perfect agreement. Furthermore, with the mass spectrometer, resolved peaks of all the natural Tin isotopes have been detected. The natural abundances extracted from these measurements are in agreement with the table values for Tin isotopes. This work, with comparison of OGE and ToF signals, confirm the fully functional SPES offline laser laboratory capability in order to develop scheme studies also for the other possible Radioactive Ion Beam (RIB) elements.

  18. Van der Waals epitaxial growth of two-dimensional single-crystalline GaSe domains on graphene

    DOE PAGES

    Li, Xufan; Basile, Leonardo; Huang, Bing; ...

    2015-07-22

    Two-dimensional (2D) van der Waals (vdW) heterostructures are a family of artificially-structured materials that promise tunable optoelectronic properties for devices with enhanced functionalities. Compared to stamping, direct epitaxy of vdW heterostructures is ideal for clean interlayer interfaces and scalable device fabrication. Here, we explore the synthesis and preferred orientations of 2D GaSe atomic layers on graphene (Gr) by vdW epitaxy. Guided by the wrinkles on graphene, GaSe nuclei form that share a predominant lattice orientation. Due to vdW epitaxial growth many nuclei grow as perfectly aligned crystals and coalesce to form large (tens of microns), single-crystal flakes. Through theoretical investigationsmore » of interlayer energetics, and measurements of preferred orientations by atomic-resolution STEM and electron diffraction, a 10.9 interlayer rotation of the GaSe lattice with respect to the underlying graphene is found to be the most energetically preferred vdW heterostructure with the largest binding energy and the longest-range ordering. These GaSe/Gr vdW heterostructures exhibit an enhanced Raman E 2 1g band of monolayer GaSe along with highly-quenched photoluminescence due to strong charge transfer. Despite the very large lattice mismatch of GaSe/Gr through vdW epitaxy, the predominant orientation control and convergent formation of large single-crystal flakes demonstrated here is promising for the scalable synthesis of large-area vdW heterostructures for the development of new optical and optoelectronic devices.« less

  19. Van der Waals epitaxial growth of two-dimensional single-crystalline GaSe domains on graphene

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Li, Xufan; Basile, Leonardo; Huang, Bing

    Two-dimensional (2D) van der Waals (vdW) heterostructures are a family of artificially-structured materials that promise tunable optoelectronic properties for devices with enhanced functionalities. Compared to stamping, direct epitaxy of vdW heterostructures is ideal for clean interlayer interfaces and scalable device fabrication. Here, we explore the synthesis and preferred orientations of 2D GaSe atomic layers on graphene (Gr) by vdW epitaxy. Guided by the wrinkles on graphene, GaSe nuclei form that share a predominant lattice orientation. Due to vdW epitaxial growth many nuclei grow as perfectly aligned crystals and coalesce to form large (tens of microns), single-crystal flakes. Through theoretical investigationsmore » of interlayer energetics, and measurements of preferred orientations by atomic-resolution STEM and electron diffraction, a 10.9 interlayer rotation of the GaSe lattice with respect to the underlying graphene is found to be the most energetically preferred vdW heterostructure with the largest binding energy and the longest-range ordering. These GaSe/Gr vdW heterostructures exhibit an enhanced Raman E 2 1g band of monolayer GaSe along with highly-quenched photoluminescence due to strong charge transfer. Despite the very large lattice mismatch of GaSe/Gr through vdW epitaxy, the predominant orientation control and convergent formation of large single-crystal flakes demonstrated here is promising for the scalable synthesis of large-area vdW heterostructures for the development of new optical and optoelectronic devices.« less

  20. TiO(2) doping by hydroxyurea at the nucleation stage: towards a new photocatalyst in the visible spectral range.

    PubMed

    Azouani, R; Tieng, S; Chhor, K; Bocquet, J-F; Eloy, P; Gaigneaux, E M; Klementiev, K; Kanaev, A V

    2010-10-07

    We report an original method of preparation of OCN-doped TiO(2) for photocatalysis in the visible spectral range. The preparation is achieved by a sol-gel route using titanium tetraisopropoxide precursor. Special attention was paid to fluid micromixing, which enables homogeneous reaction conditions in the reactor bulk and monodispersity of the produced clusters/nanoparticles. The dopant hydroxyurea (HyU, CH(4)N(2)O(2)) is injected into the reactive fluid at the nucleation stage, which lasts tens of milliseconds. The doping results in a strong yellow coloration of the nanocolloids due to the absorption band in the spectral range 380-550 nm and accelerates the aggregation kinetics of both nuclei at the induction stage and sub-nuclei units (clusters) at the nucleation stage. FTIR, Raman and UV-visible absorption analyses show the formation of a stable HyU-TiO(2) complex. EXAFS spectra indicate no appreciable changes of the first-shell Ti atom environment. The doping agent takes available surface sites of TiO(2) clusters/nanoparticles attaining ∼10% molar loading. The reaction kinetics then accelerates due to a longer collisional lifetime between nanoparticles induced by the formation of a weak [double bond, length as m-dash]OTi bond. The OCN-group bonding to titanium atoms produces a weakening of the C[double bond, length as m-dash]O double bond and a strengthening of the C-N and N-O bonds.

  1. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Allmond, J. M.; Wood, J. L.

    We extracted empirical moments of inertia, J1, J2, J3, of atomic nuclei with E(4more » $$+\\atop{1}$$)/E(2$$+\\atop{1}$$ ) > 2.7 from experimental 2$$+\\atop{g,y}$$, energies and electric quadrupole matrix elements, determined from multi- step Coulomb excitation data, and the results are compared to expectations based on rigid and irro- tational inertial flow. Only by having the signs of the E2 matrix elements, i.e., <2$$+\\atop{g}$$ ||M (E2)||2$$+\\atop{g}$$> and <0$$+\\atop{g}$$ ||M (E2)||2$$+\\atop{g}$$> < 2$$+\\atop{g}$$ ||M (E2)||2$$+\\atop{γ}$$> <2$$+\\atop{γ}$$ ||M (E2)||0$$+\\atop{g}$$> , can a unique solution to all three components of the inertia tensor of an asymmetric top be obtained. And while the absolute moments of inertia fall between the rigid and irrotational values as expected, the relative moments of inertia appear to be qualitatively consistent with the β 2 sin 2(γ ) dependence of the Bohr Hamiltonian which originates from a SO(5) in- variance. A better understanding of inertial flow is central to improving collective models, particularly hydrodynamic-based collective models. The results suggest that a better description of collective dynamics and inertial flow for atomic nuclei is needed. The inclusion of vorticity degrees of freedom may provide a path forward. This is our first report of empirical moments of inertia for all three axes and the results should challenge both collective and microscopic descriptions of inertial flow.« less

  2. Empirical mass formula with proton-neutron interaction

    NASA Astrophysics Data System (ADS)

    Tachibana, Takahiro; Uno, Masahiro; Yamada, So; Yamada, Masami

    1987-12-01

    An atomic mass formula consisting of a gross part, and averge even-odd part and an empirical shell part is studied. The gross part is, apart from a small atomic term, taken to be the sum of nucleon rest masses. Coulomb energies and a polynomial in A1/3 and ‖N-Z‖/A. The shell part includes, in addition to proton and neutron support of nuclear magicities and the cooperative deformation effect. After the first construction of such a formula, refinements have been made in two respects. One is a separate treatment of Z=N odd-odd nuclei suggested by a quartet model, and the other is an improvement of the proton neutron interaction term. By these refinements the root-mean-square deviation of calculated masses from the 1986 Audi-Wapstra masses has been reduced from 538 keV to 460 keV.

  3. Solitonic excitations in collisions of superfluid nuclei a qualitatively new phenomenon distinct from the Josephson effect

    NASA Astrophysics Data System (ADS)

    Sekizawa, Kazuyuki; Wlazłowski, Gabriel; Magierski, Piotr

    2017-11-01

    Recently, we have reported a novel role of pairing in low-energy heavy ion reactions at energies above the Coulomb barrier, which may have a detectable impact on reaction outcomes, such as the kinetic energy of fragments and the fusion cross section [arXiv:1611.10261, arXiv:1702.00069]. The phenomenon mimics the one studied experimentally with ultracold atomic gases, where two clouds of fermionic superfluids with different phases of the pairing fields are forced to merge, inducing various excitation modes of the pairing field. Although it originates from the phase difference of the pairing fields, the physics behind it is markedly different from the so-called Josephson effect. In this short contribution, we will briefly outline the results discussed in our recent papers and explain relations with the field of ultracold atomic gases.

  4. And So Ad Infinitum: The Search for Quark and Lepton Substructure

    DOE PAGES

    Lincoln, Don

    2018-04-01

    The Victorian era mathematician, Augustus de Morgan wrote, “Great fleas have little fleas upon their backs to bite ‘em, And little fleas have lesser fleas, and so ad infinitum.” This parody of Jonathan Swift’s 1733 poem On Poetry: A Rhapsody arose from a literary history, but it is rather easy to see a metaphor for nature in these words. The saga of the search for the ultimate constituents of matter has long been one of finding a seemingly fundamental structure that, in turn, was found to be made of even smaller building blocks. Matter is made of molecules. Molecules aremore » in turn made of atoms, which are themselves made of electrons and atomic nuclei. Furthermore, the nucleus consists of protons and neutrons, and these nucleons are composed of quarks.« less

  5. NMR Spectra of Oriented Samples of Intercalated Fluorographite and 19F Chemical Shielding Anisotropy of the CIF 3 Molecule

    NASA Astrophysics Data System (ADS)

    Panich, A. M.

    The analysis of 19F NMR spectra of polycrystalline and partially oriented samples of fluorinated graphite (C 2F) n intercalated with chlorine trifluoride has been carried out. Molecular mobility results in almost complete averaging of the dipole-dipole interactions of nuclei, while the essential chemical shielding anisotropy (CSA) is manifested. There is suggested molecular rotation about its C2 axes, which in turn rotates about the normal to the graphite plane. The CSA (σ || - σ ⊥) is determined to be 510 and -640 ppm, respectively, for the two inequivalent fluorine atoms of the molecule. The effect of the "antiparamagnetic" shielding leading to inversion of the chemical shielding tenser [(σ || - σ ⊥) < 0] for the equatorial F atom and anomalous line disposition in the NMR spectrum is discussed.

  6. And So Ad Infinitum: The Search for Quark and Lepton Substructure

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Lincoln, Don

    The Victorian era mathematician, Augustus de Morgan wrote, “Great fleas have little fleas upon their backs to bite ‘em, And little fleas have lesser fleas, and so ad infinitum.” This parody of Jonathan Swift’s 1733 poem On Poetry: A Rhapsody arose from a literary history, but it is rather easy to see a metaphor for nature in these words. The saga of the search for the ultimate constituents of matter has long been one of finding a seemingly fundamental structure that, in turn, was found to be made of even smaller building blocks. Matter is made of molecules. Molecules aremore » in turn made of atoms, which are themselves made of electrons and atomic nuclei. Furthermore, the nucleus consists of protons and neutrons, and these nucleons are composed of quarks.« less

  7. Direct observation of hierarchical nucleation of martensite and size-dependent superelasticity in shape memory alloys.

    PubMed

    Liu, Lifeng; Ding, Xiangdong; Li, Ju; Lookman, Turab; Sun, Jun

    2014-02-21

    Martensitic transformation usually creates hierarchical internal structures beyond mere change of the atomic crystal structure. Multi-stage nucleation is thus required, where nucleation (level-1) of the underlying atomic crystal lattice does not have to be immediately followed by the nucleation of higher-order superstructures (level-2 and above), such as polysynthetic laths. Using in situ transmission electron microscopy (TEM), we directly observe the nucleation of the level-2 superstructure in a Cu-Al-Ni single crystal under compression, with critical super-nuclei size L2c around 500 nm. When the sample size D decreases below L2c, the superelasticity behavior changes from a flat stress plateau to a continuously rising stress-strain curve. Such size dependence definitely would impact the application of shape memory alloys in miniaturized MEMS/NEMS devices.

  8. The electron screening puzzle and nuclear clustering

    DOE PAGES

    Spitaleri, C.; Bertulani, C. A.; Fortunato, L.; ...

    2016-02-12

    Accurate measurements of nuclear reactions of astrophysical interest within, or close to, the Gamow peak show evidence of an unexpected effect attributed to the presence of atomic electrons in the target. The experiments need to include an effective "screening" potential to explain the enhancement of the cross sections at the lowest measurable energies. Despite various theoretical studies conducted over the past 20 years and numerous experimental measurements, a theory has not yet been found that can explain the cause of the exceedingly high values of the screening potential needed to explain the data. Furthermore, in this letter we show thatmore » instead of an atomic physics solution of the "electron screening puzzle", the reason for the large screening potential values is in fact due to clusterization effects in nuclear reactions, in particular for reaction involving light nuclei.« less

  9. Origin and propagation of galactic cosmic rays

    NASA Technical Reports Server (NTRS)

    Cesarsky, Catherine J.; Ormes, Jonathan F.

    1987-01-01

    The study of systematic trends in elemental abundances is important for unfolding the nuclear and/or atomic effects that should govern the shaping of source abundances and in constraining the parameters of cosmic ray acceleration models. In principle, much can be learned about the large-scale distributions of cosmic rays in the galaxy from all-sky gamma ray surveys such as COS-B and SAS-2. Because of the uncertainties in the matter distribution which come from the inability to measure the abundance of molecular hydrogen, the results are somewhat controversial. The leaky-box model accounts for a surprising amount of the data on heavy nuclei. However, a growing body of data indicates that the simple picture may have to be abandoned in favor of more complex models which contain additional parameters. Future experiments on the Spacelab and space station will hopefully be made of the spectra of individual nuclei at high energy. Antiprotons must be studied in the background free environment above the atmosphere with much higher reliability and presion to obtain spectral information.

  10. Beta-spectrum shapes of forbidden β decays

    NASA Astrophysics Data System (ADS)

    Kostensalo, Joel; Suhonen, Jouni

    2018-03-01

    The neutrinoless ββ decay of atomic nuclei continues to attract fervent interest due to its potential to confirm the possible Majorana nature of the neutrino, and thus the nonconservation of the lepton number. At the same time, the direct dark matter experiments are looking for weakly interacting massive particles (WIMPs) through their scattering on nuclei. The neutrino-oscillation experiments on reactor antineutrinos base their analyses on speculations of β-spectrum shapes of nuclear decays, thus leading to the notorious “reactor antineutrino anomaly.” In all these experimental efforts, one encounters the problem of β-spectrum shapes of forbidden β decays, either as unwanted backgrounds or unknown components in the analyses of data. In this work, the problem of spectrum shapes is discussed and illustrated with a set of selected examples. The relation of the β-spectrum shapes to the problem of the effective value of the weak axial-vector coupling strength gA and the enhancement of the axial-charge matrix element is also pointed out.

  11. Quantum nature of protons in water probed by scanning tunneling microscopy and spectroscopy

    NASA Astrophysics Data System (ADS)

    Guo, Jing; Lü, Jing-Tao; Feng, Yexin; Chen, Ji; Peng, Jinbo; Lin, Zeren; Meng, Xiangzhi; Wang, Zhichang; Li, Xin-Zheng; Wang, En-Ge; Jiang, Ying; Jing-Tao Lü Team; Xin-Zheng Li Team

    The complexity of hydrogen-bonding interaction largely arises from the quantum nature of light hydrogen nuclei, which has remained elusive for decades. Here we report the direct assessment of nuclear quantum effects on the strength of a single hydrogen bond formed at a water-salt interface, using tip-enhanced inelastic electron tunneling spectroscopy (IETS) based on a low-temperature scanning tunneling microscope (STM). The IETS signals are resonantly enhanced by gating the frontier orbitals of water via a chlorine-terminated STM tip, such that the hydrogen-bonding strength can be determined with unprecedentedly high accuracy from the redshift in the O-H stretching frequency of water. Isotopic substitution experiments combined with quantum simulations reveal that the anharmonic quantum fluctuations of hydrogen nuclei weaken the weak hydrogen bonds and strengthen the relatively strong ones. However, this trend can be completely reversed when the hydrogen bond is strongly coupled to the polar atomic sites of the surface.

  12. Measurement of Recoil Losses and Ranges for Spallation Products Produced in Proton Interactions with Al, Si, Mg at 200 and 500 MeV

    NASA Technical Reports Server (NTRS)

    Sisterson, J. M.

    2005-01-01

    Cosmic rays interact with extraterrestrial materials to produce a variety of spallation products. If these cosmogenic nuclides are produced within an inclusion in such material, then an important consideration is the loss of the product nuclei, which recoil out of the inclusion. Of course, at the same time, some atoms of the product nuclei under study may be knocked into the inclusion from the surrounding material, which is likely to have a different composition to that of the inclusion [1]. For example, Ne-21 would be produced in presolar grains, such as SiC, when irradiated in interstellar space. However, to calculate a presolar age, one needs to know how much 21Ne is retained in the grain. For small grains, the recoil losses might be large [2, 3] To study this effect under laboratory conditions, recoil measurements were made using protons with energies from 66 - 1600 MeV on Si, Al and Ba targets [3, 4, 5].

  13. Nuclear Dependence of the Transverse-Single-Spin Asymmetry for Forward Neutron Production in Polarized p +A Collisions at √{sN N}=200 GeV

    NASA Astrophysics Data System (ADS)

    Aidala, C.; Akiba, Y.; Alfred, M.; Andrieux, V.; Aoki, K.; Apadula, N.; Asano, H.; Ayuso, C.; Azmoun, B.; Babintsev, V.; Bagoly, A.; Bandara, N. S.; Barish, K. N.; Bathe, S.; Bazilevsky, A.; Beaumier, M.; Belmont, R.; Berdnikov, A.; Berdnikov, Y.; Blau, D. S.; Boer, M.; Bok, J. S.; Brooks, M. L.; Bryslawskyj, J.; Bumazhnov, V.; Butler, C.; Campbell, S.; Canoa Roman, V.; Cervantes, R.; Chi, C. Y.; Chiu, M.; Choi, I. J.; Choi, J. B.; Citron, Z.; Connors, M.; Cronin, N.; Csanád, M.; Csörgő, T.; Danley, T. W.; Daugherity, M. S.; David, G.; Deblasio, K.; Dehmelt, K.; Denisov, A.; Deshpande, A.; Desmond, E. J.; Dion, A.; Dixit, D.; Do, J. H.; Drees, A.; Drees, K. A.; Dumancic, M.; Durham, J. M.; Durum, A.; Elder, T.; Enokizono, A.; En'yo, H.; Esumi, S.; Fadem, B.; Fan, W.; Feege, N.; Fields, D. E.; Finger, M.; Finger, M.; Fokin, S. L.; Frantz, J. E.; Franz, A.; Frawley, A. D.; Fukuda, Y.; Gal, C.; Gallus, P.; Garg, P.; Ge, H.; Giordano, F.; Goto, Y.; Grau, N.; Greene, S. V.; Grosse Perdekamp, M.; Gunji, T.; Guragain, H.; Hachiya, T.; Haggerty, J. S.; Hahn, K. I.; Hamagaki, H.; Hamilton, H. F.; Han, S. Y.; Hanks, J.; Hasegawa, S.; Haseler, T. O. S.; He, X.; Hemmick, T. K.; Hill, J. C.; Hill, K.; Hollis, R. S.; Homma, K.; Hong, B.; Hoshino, T.; Hotvedt, N.; Huang, J.; Huang, S.; Imai, K.; Imrek, J.; Inaba, M.; Iordanova, A.; Isenhower, D.; Ito, Y.; Ivanishchev, D.; Jacak, B. V.; Jezghani, M.; Ji, Z.; Jiang, X.; Johnson, B. M.; Jorjadze, V.; Jouan, D.; Jumper, D. S.; Kang, J. H.; Kapukchyan, D.; Karthas, S.; Kawall, D.; Kazantsev, A. V.; Khachatryan, V.; Khanzadeev, A.; Kim, C.; Kim, D. J.; Kim, E.-J.; Kim, M.; Kim, M. H.; Kincses, D.; Kistenev, E.; Klatsky, J.; Kline, P.; Koblesky, T.; Kotov, D.; Kudo, S.; Kurita, K.; Kwon, Y.; Lajoie, J. G.; Lallow, E. O.; Lebedev, A.; Lee, S.; Leitch, M. J.; Leung, Y. H.; Lewis, N. A.; Li, X.; Lim, S. H.; Liu, L. D.; Liu, M. X.; Loggins, V.-R.; Lökös, S.; Lovasz, K.; Lynch, D.; Majoros, T.; Makdisi, Y. I.; Makek, M.; Malaev, M.; Manko, V. I.; Mannel, E.; Masuda, H.; McCumber, M.; McGaughey, P. L.; McGlinchey, D.; McKinney, C.; Mendoza, M.; Metzger, W. J.; Mignerey, A. C.; Mihalik, D. E.; Milov, A.; Mishra, D. K.; Mitchell, J. T.; Mitsuka, G.; Miyasaka, S.; Mizuno, S.; Montuenga, P.; Moon, T.; Morrison, D. P.; Morrow, S. I. M.; Murakami, T.; Murata, J.; Nagai, K.; Nagashima, K.; Nagashima, T.; Nagle, J. L.; Nagy, M. I.; Nakagawa, I.; Nakagomi, H.; Nakano, K.; Nattrass, C.; Niida, T.; Nouicer, R.; Novák, T.; Novitzky, N.; Novotny, R.; Nyanin, A. S.; O'Brien, E.; Ogilvie, C. A.; Orjuela Koop, J. D.; Osborn, J. D.; Oskarsson, A.; Ottino, G. J.; Ozawa, K.; Pantuev, V.; Papavassiliou, V.; Park, J. S.; Park, S.; Pate, S. F.; Patel, M.; Peng, W.; Perepelitsa, D. V.; Perera, G. D. N.; Peressounko, D. Yu.; Perezlara, C. E.; Perry, J.; Petti, R.; Phipps, M.; Pinkenburg, C.; Pisani, R. P.; Pun, A.; Purschke, M. L.; Radzevich, P. V.; Read, K. F.; Reynolds, D.; Riabov, V.; Riabov, Y.; Richford, D.; Rinn, T.; Rolnick, S. D.; Rosati, M.; Rowan, Z.; Runchey, J.; Safonov, A. S.; Sakaguchi, T.; Sako, H.; Samsonov, V.; Sarsour, M.; Sato, K.; Sato, S.; Schaefer, B.; Schmoll, B. K.; Sedgwick, K.; Seidl, R.; Sen, A.; Seto, R.; Sexton, A.; Sharma, D.; Shein, I.; Shibata, T.-A.; Shigaki, K.; Shimomura, M.; Shioya, T.; Shukla, P.; Sickles, A.; Silva, C. L.; Silvermyr, D.; Singh, B. K.; Singh, C. P.; Singh, V.; Skoby, M. J.; Slunečka, M.; Smith, K. L.; Snowball, M.; Soltz, R. A.; Sondheim, W. E.; Sorensen, S. P.; Sourikova, I. V.; Stankus, P. W.; Stoll, S. P.; Sugitate, T.; Sukhanov, A.; Sumita, T.; Sun, J.; Syed, S.; Sziklai, J.; Takeda, A.; Tanida, K.; Tannenbaum, M. J.; Tarafdar, S.; Taranenko, A.; Tarnai, G.; Tieulent, R.; Timilsina, A.; Todoroki, T.; Tomášek, M.; Towell, C. L.; Towell, R. S.; Tserruya, I.; Ueda, Y.; Ujvari, B.; van Hecke, H. W.; Vazquez-Carson, S.; Velkovska, J.; Virius, M.; Vrba, V.; Vukman, N.; Wang, X. R.; Wang, Z.; Watanabe, Y.; Watanabe, Y. S.; Wong, C. P.; Woody, C. L.; Xu, C.; Xu, Q.; Xue, L.; Yalcin, S.; Yamaguchi, Y. L.; Yamamoto, H.; Yanovich, A.; Yin, P.; Yoo, J. H.; Yoon, I.; Yu, H.; Yushmanov, I. E.; Zajc, W. A.; Zelenski, A.; Zharko, S.; Zou, L.; Phenix Collaboration

    2018-01-01

    During 2015, the Relativistic Heavy Ion Collider (RHIC) provided collisions of transversely polarized protons with Au and Al nuclei for the first time, enabling the exploration of transverse-single-spin asymmetries with heavy nuclei. Large single-spin asymmetries in very forward neutron production have been previously observed in transversely polarized p +p collisions at RHIC, and the existing theoretical framework that was successful in describing the single-spin asymmetry in p +p collisions predicts only a moderate atomic-mass-number (A ) dependence. In contrast, the asymmetries observed at RHIC in p +A collisions showed a surprisingly strong A dependence in inclusive forward neutron production. The observed asymmetry in p +Al collisions is much smaller, while the asymmetry in p +Au collisions is a factor of 3 larger in absolute value and of opposite sign. The interplay of different neutron production mechanisms is discussed as a possible explanation of the observed A dependence.

  14. Nuclear Dependence of the Transverse-Single-Spin Asymmetry for Forward Neutron Production in Polarized p+A Collisions at sqrt[s_{NN}]=200  GeV.

    PubMed

    Aidala, C; Akiba, Y; Alfred, M; Andrieux, V; Aoki, K; Apadula, N; Asano, H; Ayuso, C; Azmoun, B; Babintsev, V; Bagoly, A; Bandara, N S; Barish, K N; Bathe, S; Bazilevsky, A; Beaumier, M; Belmont, R; Berdnikov, A; Berdnikov, Y; Blau, D S; Boer, M; Bok, J S; Brooks, M L; Bryslawskyj, J; Bumazhnov, V; Butler, C; Campbell, S; Canoa Roman, V; Cervantes, R; Chi, C Y; Chiu, M; Choi, I J; Choi, J B; Citron, Z; Connors, M; Cronin, N; Csanád, M; Csörgő, T; Danley, T W; Daugherity, M S; David, G; DeBlasio, K; Dehmelt, K; Denisov, A; Deshpande, A; Desmond, E J; Dion, A; Dixit, D; Do, J H; Drees, A; Drees, K A; Dumancic, M; Durham, J M; Durum, A; Elder, T; Enokizono, A; En'yo, H; Esumi, S; Fadem, B; Fan, W; Feege, N; Fields, D E; Finger, M; Finger, M; Fokin, S L; Frantz, J E; Franz, A; Frawley, A D; Fukuda, Y; Gal, C; Gallus, P; Garg, P; Ge, H; Giordano, F; Goto, Y; Grau, N; Greene, S V; Grosse Perdekamp, M; Gunji, T; Guragain, H; Hachiya, T; Haggerty, J S; Hahn, K I; Hamagaki, H; Hamilton, H F; Han, S Y; Hanks, J; Hasegawa, S; Haseler, T O S; He, X; Hemmick, T K; Hill, J C; Hill, K; Hollis, R S; Homma, K; Hong, B; Hoshino, T; Hotvedt, N; Huang, J; Huang, S; Imai, K; Imrek, J; Inaba, M; Iordanova, A; Isenhower, D; Ito, Y; Ivanishchev, D; Jacak, B V; Jezghani, M; Ji, Z; Jiang, X; Johnson, B M; Jorjadze, V; Jouan, D; Jumper, D S; Kang, J H; Kapukchyan, D; Karthas, S; Kawall, D; Kazantsev, A V; Khachatryan, V; Khanzadeev, A; Kim, C; Kim, D J; Kim, E-J; Kim, M; Kim, M H; Kincses, D; Kistenev, E; Klatsky, J; Kline, P; Koblesky, T; Kotov, D; Kudo, S; Kurita, K; Kwon, Y; Lajoie, J G; Lallow, E O; Lebedev, A; Lee, S; Leitch, M J; Leung, Y H; Lewis, N A; Li, X; Lim, S H; Liu, L D; Liu, M X; Loggins, V-R; Lökös, S; Lovasz, K; Lynch, D; Majoros, T; Makdisi, Y I; Makek, M; Malaev, M; Manko, V I; Mannel, E; Masuda, H; McCumber, M; McGaughey, P L; McGlinchey, D; McKinney, C; Mendoza, M; Metzger, W J; Mignerey, A C; Mihalik, D E; Milov, A; Mishra, D K; Mitchell, J T; Mitsuka, G; Miyasaka, S; Mizuno, S; Montuenga, P; Moon, T; Morrison, D P; Morrow, S I M; Murakami, T; Murata, J; Nagai, K; Nagashima, K; Nagashima, T; Nagle, J L; Nagy, M I; Nakagawa, I; Nakagomi, H; Nakano, K; Nattrass, C; Niida, T; Nouicer, R; Novák, T; Novitzky, N; Novotny, R; Nyanin, A S; O'Brien, E; Ogilvie, C A; Orjuela Koop, J D; Osborn, J D; Oskarsson, A; Ottino, G J; Ozawa, K; Pantuev, V; Papavassiliou, V; Park, J S; Park, S; Pate, S F; Patel, M; Peng, W; Perepelitsa, D V; Perera, G D N; Peressounko, D Yu; PerezLara, C E; Perry, J; Petti, R; Phipps, M; Pinkenburg, C; Pisani, R P; Pun, A; Purschke, M L; Radzevich, P V; Read, K F; Reynolds, D; Riabov, V; Riabov, Y; Richford, D; Rinn, T; Rolnick, S D; Rosati, M; Rowan, Z; Runchey, J; Safonov, A S; Sakaguchi, T; Sako, H; Samsonov, V; Sarsour, M; Sato, K; Sato, S; Schaefer, B; Schmoll, B K; Sedgwick, K; Seidl, R; Sen, A; Seto, R; Sexton, A; Sharma, D; Shein, I; Shibata, T-A; Shigaki, K; Shimomura, M; Shioya, T; Shukla, P; Sickles, A; Silva, C L; Silvermyr, D; Singh, B K; Singh, C P; Singh, V; Skoby, M J; Slunečka, M; Smith, K L; Snowball, M; Soltz, R A; Sondheim, W E; Sorensen, S P; Sourikova, I V; Stankus, P W; Stoll, S P; Sugitate, T; Sukhanov, A; Sumita, T; Sun, J; Syed, S; Sziklai, J; Takeda, A; Tanida, K; Tannenbaum, M J; Tarafdar, S; Taranenko, A; Tarnai, G; Tieulent, R; Timilsina, A; Todoroki, T; Tomášek, M; Towell, C L; Towell, R S; Tserruya, I; Ueda, Y; Ujvari, B; van Hecke, H W; Vazquez-Carson, S; Velkovska, J; Virius, M; Vrba, V; Vukman, N; Wang, X R; Wang, Z; Watanabe, Y; Watanabe, Y S; Wong, C P; Woody, C L; Xu, C; Xu, Q; Xue, L; Yalcin, S; Yamaguchi, Y L; Yamamoto, H; Yanovich, A; Yin, P; Yoo, J H; Yoon, I; Yu, H; Yushmanov, I E; Zajc, W A; Zelenski, A; Zharko, S; Zou, L

    2018-01-12

    During 2015, the Relativistic Heavy Ion Collider (RHIC) provided collisions of transversely polarized protons with Au and Al nuclei for the first time, enabling the exploration of transverse-single-spin asymmetries with heavy nuclei. Large single-spin asymmetries in very forward neutron production have been previously observed in transversely polarized p+p collisions at RHIC, and the existing theoretical framework that was successful in describing the single-spin asymmetry in p+p collisions predicts only a moderate atomic-mass-number (A) dependence. In contrast, the asymmetries observed at RHIC in p+A collisions showed a surprisingly strong A dependence in inclusive forward neutron production. The observed asymmetry in p+Al collisions is much smaller, while the asymmetry in p+Au collisions is a factor of 3 larger in absolute value and of opposite sign. The interplay of different neutron production mechanisms is discussed as a possible explanation of the observed A dependence.

  15. A rare-earth-magnet ion trap for confining low-Z, bare nuclei

    NASA Astrophysics Data System (ADS)

    Brewer, Samuel M.; Tan, Joseph N.

    2009-05-01

    Simplifications in the theory for Rydberg states of hydrogenlike ions allow a substantial improvement in the accuracy of predicted levels, which can yield information on the values of fundamental constants and test theory if they can be compared with precision frequency measurements.[1] We consider the trapping of bare nuclei (fully-stripped) to be used in making Rydberg states of one-electron ions with atomic number 1< Z < 11. Numerical simulation is used here to study ion confinement in a compact, Penning-style ion trap consisting of electrodes integrated with rare-earth permanent magnets, and to model the capture of charge-state-selected ions extracted from an electron beam ion trap (EBIT). An experimental apparatus adapted to the NIST EBIT will also be discussed. Reference: [1] U.D. Jentschura, P.J. Mohr, J.N. Tan, and B.J. Wundt, ``Fundamental constants and tests of theory in Rydberg states of hydrogenlike ions,'' Phys. Rev. Lett. 100, 160404 (2008).

  16. Targets used in the production of radioactive ion beams at the HRIBF

    NASA Astrophysics Data System (ADS)

    Stracener, D. W.; Alton, G. D.; Auble, R. L.; Beene, J. R.; Mueller, P. E.; Bilheux, J. C.

    2004-03-01

    Radioactive ion beams are produced at the Holifield Radioactive Ion Beam Facility using the Isotope Separation On-Line (ISOL) technique where the atoms are produced in a thick target, transported to an ion source, ionized, and extracted from the ion source to form an ion beam. These radioactive ion beams are then accelerated to energies of a few MeV per nucleon and delivered to experimental stations for use in nuclear physics and nuclear astrophysics experiments. At the heart of this facility is the RIB production target, where the radioactive nuclei are produced using beams of light ions (p, d, 3He, α) to induce nuclear reactions in the target nuclei. Several target materials have been developed and used successfully, including Al 2O 3, HfO 2, SiC, CeS, liquid Ge, liquid Ni, and a low-density matrix of uranium carbide. The details of these targets and some of the target developments that led to the delivery of high-quality radioactive ion beams are discussed in this paper.

  17. Study of Light Neutron-Rich Nuclei Using a Multilayer Semiconductor Setup

    NASA Astrophysics Data System (ADS)

    Gurov, Yu. B.; Lapushkin, S. V.; Sandukovsky, V. G.; Chernyshev, B. A.

    2017-12-01

    The characteristics of two modifications of the semiconductor (s.c.d.) setup consisting of telescopes on the basis of silicon detectors are presented. These settings allow performing a precision measurement of energy in a large dynamic range (from a few to hundreds of MeV) and particle identification in a wide range of masses. The issues of measurement of the characteristics of s.c.d. telescopes and their impact on the quality of the obtained experimental data are considered. Considerable attention is paid to the use of created semiconductor devices for the search for and spectroscopy of light exotic nuclei on the accelerators of PNPI (Gatchina) and LANL (Los Alamos).

  18. Monte-Carlo gamma response simulation of fast/thermal neutron interactions with soil elements

    USDA-ARS?s Scientific Manuscript database

    Soil elemental analysis using characteristic gamma rays induced by neutrons is an effective method of in situ soil content determination. The nuclei of soil elements irradiated by neutrons issue characteristic gamma rays due to both inelastic neutron scattering (e.g., Si, C) and thermal neutron capt...

  19. Mössbauer spectroscopy and the structure of interfaces on the atomic scale in metallic nanosystems

    NASA Astrophysics Data System (ADS)

    Uzdin, V. M.

    2007-10-01

    A microscopic model of the formation of an alloy on the interface has been constructed, which takes into account the exchange of atoms with the substrate atoms and the “floating up” of the latter into the upper layers in the process of epitaxial growth. The self-consistent calculations of atomic magnetic moments of spatially inhomogeneous structures obtained in this case are used for the interpretation of data of Mössbauer spectroscopy. The proposed scenario of mixing leads to the appearance of a preferred direction in the sample and the asymmetry of interfaces in the direction of epitaxial growth. In the multilayer M 1/ M 2 ( M 1,2 = Fe, Cr, V, Sn, or Ag) systems, this asymmetry makes it possible to understand the difference in the magnetic behavior of M 1-on M 2 and M 2-on- M 1 interfaces which has been observed experimentally. The correlation between the calculated distributions of magnetic moments and the measured distributions of hyperfine fields at iron atoms confirms the assumption about their proportionality for a broad class of metallic multilayer systems. However, a linear decrease of hyperfine fields at the 57Fe nuclei with increasing number of impurity atoms among the nearest and next-nearest neighbors is not confirmed for Fe/Cr systems, although is correct in Fe/V superlattices. In the Fe/Cr multilayer systems, the experimentally measured value of magnetoresistance grows with increasing fraction of the “floated up” atoms of 57Fe. Thus, it is the bulk scattering by impurity atoms that gives the basic contribution to the effect of giant magnetoresistance. The problem of the influence of mixing and adsorption of hydrogen in the vanadium layers on the state of the spin-density wave in V/Cr superlattices has been considered.

  20. Local configurations and atomic intermixing in as-quenched and annealed Fe1-xCrx and Fe1-xMox ribbons

    NASA Astrophysics Data System (ADS)

    Stanciu, A. E.; Greculeasa, S. G.; Bartha, C.; Schinteie, G.; Palade, P.; Kuncser, A.; Leca, A.; Filoti, G.; Birsan, A.; Crisan, O.; Kuncser, V.

    2018-04-01

    Local atomic configuration, phase composition and atomic intermixing in Fe-rich Fe1-xCrx and Fe1-xMox ribbons (x = 0.05, 0.10, 0.15), of potential interest for high-temperature applications and nuclear devices, are investigated in this study in relation to specific processing and annealing routes. The Fe-based thin ribbons have been prepared by induction melting, followed by melt spinning and further annealed in He at temperatures up to 1250 °C. The complex structural, compositional and atomic configuration characterisation has been performed by means of X-ray diffraction (XRD), transmission Mössbauer spectroscopy and differential scanning calorimetry (TG-DSC). The XRD analysis indicates the formation of the desired solid solutions with body-centred cubic (bcc) structure in the as-quenched state. The Mössbauer spectroscopy results have been analysed in terms of the two-shell model. The distribution of Cr/Mo atoms in the first two coordination spheres is not homogeneous, especially after annealing, as supported by the short-range order parameters. In addition, high-temperature annealing treatments give rise to oxidation of Fe (to haematite, maghemite and magnetite) at the surface of the ribbons. Fe1-xCrx alloys are structurally more stable than the Mo counterpart under annealing at 700 °C. Annealing at 1250 °C in He enhances drastically the Cr clustering around Fe nuclei.

  1. Study of photon emission by electron capture during solar nuclei acceleration, 1: Temperature-dependent cross section for charge changing processes

    NASA Technical Reports Server (NTRS)

    Perez-Peraza, J.; Alvarez, M.; Laville, A.; Gallegos, A.

    1985-01-01

    The study of charge changing cross sections of fast ions colliding with matter provides the fundamental basis for the analysis of the charge states produced in such interactions. Given the high degree of complexity of the phenomena, there is no theoretical treatment able to give a comprehensive description. In fact, the involved processes are very dependent on the basic parameters of the projectile, such as velocity charge state, and atomic number, and on the target parameters, the physical state (molecular, atomic or ionized matter) and density. The target velocity, may have also incidence on the process, through the temperature of the traversed medium. In addition, multiple electron transfer in single collisions intrincates more the phenomena. Though, in simplified cases, such as protons moving through atomic hydrogen, considerable agreement has been obtained between theory and experiments However, in general the available theoretical approaches have only limited validity in restricted regions of the basic parameters. Since most measurements of charge changing cross sections are performed in atomic matter at ambient temperature, models are commonly based on the assumption of targets at rest, however at Astrophysical scales, temperature displays a wide range in atomic and ionized matter. Therefore, due to the lack of experimental data , an attempt is made here to quantify temperature dependent cross sections on basis to somewhat arbitrary, but physically reasonable assumptions.

  2. Highlights in light-baryon spectroscopy and searches for gluonic excitations

    NASA Astrophysics Data System (ADS)

    Crede, Volker

    2016-01-01

    The spectrum of excited hadrons - mesons and baryons - serves as an excellent probe of quantum chromodynamics (QCD), the fundamental theory of the strong interaction. The strong coupling however makes QCD challenging. It confines quarks and breaks chiral symmetry, thus providing us with the world of light hadrons. Highly-excited hadronic states are sensitive to the details of quark confinement, which is only poorly understood within QCD. This is the regime of non-perturbative QCD and it is one of the key issues in hadronic physics to identify the corresponding internal degrees of freedom and how they relate to strong coupling QCD. The quark model suggests mesons are made of a constituent quark and an antiquark and baryons consist of three such quarks. QCD predicts other forms of matter. What is the role of glue? Resonances with large gluonic components are predicted as bound states by QCD. The lightest hybrid mesons with exotic quantum numbers are estimated to have masses in the range from 1 to 2 GeV/c2 and are well in reach of current experimental programs. At Jefferson Laboratory (JLab) and other facilities worldwide, the high-energy electron and photon beams present a remarkably clean probe of hadronic matter, providing an excellent microscope for examining atomic nuclei and the strong nuclear force.

  3. A fast - Monte Carlo toolkit on GPU for treatment plan dose recalculation in proton therapy

    NASA Astrophysics Data System (ADS)

    Senzacqua, M.; Schiavi, A.; Patera, V.; Pioli, S.; Battistoni, G.; Ciocca, M.; Mairani, A.; Magro, G.; Molinelli, S.

    2017-10-01

    In the context of the particle therapy a crucial role is played by Treatment Planning Systems (TPSs), tools aimed to compute and optimize the tratment plan. Nowadays one of the major issues related to the TPS in particle therapy is the large CPU time needed. We developed a software toolkit (FRED) for reducing dose recalculation time by exploiting Graphics Processing Units (GPU) hardware. Thanks to their high parallelization capability, GPUs significantly reduce the computation time, up to factor 100 respect to a standard CPU running software. The transport of proton beams in the patient is accurately described through Monte Carlo methods. Physical processes reproduced are: Multiple Coulomb Scattering, energy straggling and nuclear interactions of protons with the main nuclei composing the biological tissues. FRED toolkit does not rely on the water equivalent translation of tissues, but exploits the Computed Tomography anatomical information by reconstructing and simulating the atomic composition of each crossed tissue. FRED can be used as an efficient tool for dose recalculation, on the day of the treatment. In fact it can provide in about one minute on standard hardware the dose map obtained combining the treatment plan, earlier computed by the TPS, and the current patient anatomic arrangement.

  4. Upper bound dose values for meson radiation in heavy-ion therapy.

    PubMed

    Rabin, C; Gonçalves, M; Duarte, S B; González-Sprinberg, G A

    2018-06-01

    Radiation treatment of cancer has evolved to include massive particle beams, instead of traditional irradiation procedures. Thus, patient doses and worker radiological protection have become issues of constant concern in the use of these new technologies, especially for proton- and heavy-ion-therapy. In the beam energies of interest of heavy-ion-therapy, secondary particle radiation comes from proton, neutron, and neutral and charged pions produced in the nuclear collisions of the beam with human tissue atoms. This work, for the first time, offers the upper bound of meson radiation dose in organic tissues due to secondary meson radiation in heavy-ion therapy. A model based on intranuclear collision has been used to follow in time the nuclear reaction and to determine the secondary radiation due to the meson yield produced in the beam interaction with nuclei in the tissue-equivalent media and water. The multiplicity, energy spectrum, and angular distribution of these pions, as well as their decay products, have been calculated in different scenarios for the nuclear reaction mechanism. The results of the produced secondary meson particles has been used to estimate the energy deposited in tissue using a cylindrical phantom by a transport Monte Carlo simulation and we have concluded that these mesons contribute at most 0.1% of the total prescribed dose.

  5. Electronic torsional sound in linear atomic chains: Chemical energy transport at 1000 km/s

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kurnosov, Arkady A.; Rubtsov, Igor V.; Maksymov, Andrii O.

    2016-07-21

    We investigate entirely electronic torsional vibrational modes in linear cumulene chains. The carbon nuclei of a cumulene are positioned along the primary axis so that they can participate only in the transverse and longitudinal motions. However, the interatomic electronic clouds behave as a torsion spring with remarkable torsional stiffness. The collective dynamics of these clouds can be described in terms of electronic vibrational quanta, which we name torsitons. It is shown that the group velocity of the wavepacket of torsitons is much higher than the typical speed of sound, because of the small mass of participating electrons compared to themore » atomic mass. For the same reason, the maximum energy of the torsitons in cumulenes is as high as a few electronvolts, while the minimum possible energy is evaluated as a few hundred wavenumbers and this minimum is associated with asymmetry of zero point atomic vibrations. Theory predictions are consistent with the time-dependent density functional theory calculations. Molecular systems for experimental evaluation of the predictions are proposed.« less

  6. A generalized any particle propagator theory: Assessment of nuclear quantum effects on electron propagator calculations

    NASA Astrophysics Data System (ADS)

    Romero, Jonathan; Posada, Edwin; Flores-Moreno, Roberto; Reyes, Andrés

    2012-08-01

    In this work we propose an extended propagator theory for electrons and other types of quantum particles. This new approach has been implemented in the LOWDIN package and applied to sample calculations of atomic and small molecular systems to determine its accuracy and performance. As a first application of the method we have studied the nuclear quantum effects on electron ionization energies. We have observed that ionization energies of atoms are similar to those obtained with the electron propagator approach. However, for molecular systems containing hydrogen atoms there are improvements in the quality of the results with the inclusion of nuclear quantum effects. An energy term analysis has allowed us to conclude that nuclear quantum effects are important for zero order energies whereas propagator results correct the electron and electron-nuclear correlation terms. Results presented for a series of n-alkanes have revealed the potential of this method for the accurate calculation of ionization energies of a wide variety of molecular systems containing hydrogen nuclei. The proposed methodology will also be applicable to exotic molecular systems containing positrons or muons.

  7. Selective absorption processes as the origin of puzzling spectral line polarization from the Sun.

    PubMed

    Trujillo Bueno, J; Landi Degl'Innocenti, E; Collados, M; Merenda, L; Manso Sainz, R

    2002-01-24

    Magnetic fields play a key role in most astrophysical systems, from the Sun to active galactic nuclei. They can be studied through their effects on atomic energy levels, which produce polarized spectral lines. In particular, anisotropic radiation 'pumping' processes (which send electrons to higher atomic levels) induce population imbalances that are modified by weak magnetic fields. Here we report peculiarly polarized light in the He I 10,830-A multiplet observed in a coronal filament located at the centre of the solar disk. We show that the polarized light arises from selective absorption from the ground level of the triplet system of helium, and that it implies the presence of magnetic fields of the order of a few gauss that are highly inclined with respect to the solar radius vector. This disproves the common belief that population imbalances in long-lived atomic levels are insignificant in the presence of inclined fields of the order of a few gauss, and opens up a new diagnostic window for the investigation of solar magnetic fields.

  8. Semi-exact concentric atomic density fitting: Reduced cost and increased accuracy compared to standard density fitting

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hollman, David S.; Department of Chemistry, Virginia Tech, Blacksburg, Virginia 24061; Schaefer, Henry F.

    2014-02-14

    A local density fitting scheme is considered in which atomic orbital (AO) products are approximated using only auxiliary AOs located on one of the nuclei in that product. The possibility of variational collapse to an unphysical “attractive electron” state that can affect such density fitting [P. Merlot, T. Kjærgaard, T. Helgaker, R. Lindh, F. Aquilante, S. Reine, and T. B. Pedersen, J. Comput. Chem. 34, 1486 (2013)] is alleviated by including atom-wise semidiagonal integrals exactly. Our approach leads to a significant decrease in the computational cost of density fitting for Hartree–Fock theory while still producing results with errors 2–5 timesmore » smaller than standard, nonlocal density fitting. Our method allows for large Hartree–Fock and density functional theory computations with exact exchange to be carried out efficiently on large molecules, which we demonstrate by benchmarking our method on 200 of the most widely used prescription drug molecules. Our new fitting scheme leads to smooth and artifact-free potential energy surfaces and the possibility of relatively simple analytic gradients.« less

  9. Studies of the Interaction of Influenza Virus RNA Polymerase PAN with Endonuclease Inhibitors.

    PubMed

    Dong, Li-Hua; Cao, Xiao-Rong

    2018-06-01

    Influenza virus is a major causative agent of respiratory viral infections, and RNA polymerase catalyzes its replication and transcription activities in infected cell nuclei. Since it is highly conserved in all virus strains, RNA polymerase becomes a key target of anti-influenza virus agents. Although experimental studies have revealed the good inhibitory activity of endonuclease inhibitors to RNA polymerase, the mechanism is still unclear. In this study, the docking and molecular dynamics simulations have been performed to explore the interaction of three kinds of endonuclease inhibitors with the subunit (PA N ) of RNA polymerase. Our calculations indicate that all these endonuclease inhibitors can bind to the binding pocket of PA N , in which the electronegative oxygen atoms of the inhibitors form a chelated structure with the two Mn 2+ cations of the active center. The most important interaction between these inhibitors and PA N is electrostatic interaction. The electron density of the chelate oxygen atoms determines the magnitude of the electrostatic energy, and the chelated structure and orientation of inhibitors depend largely on the distance between the chelate oxygen atoms.

  10. Mass predictions of atomic nuclei in the infinite nuclear matter model

    NASA Astrophysics Data System (ADS)

    Nayak, R. C.; Satpathy, L.

    2012-07-01

    We present here the mass excesses, binding energies, one- and two-neutron, one- and two-proton and α-particle separation energies of 6727 nuclei in the ranges 4≤Z≤120 and 8≤A≤303 calculated in the infinite nuclear matter model. Compared to our predictions of 1999 mass table, the present ones are obtained using larger data base of 2003 mass table of Wapstra and Audi and resorting to higher accuracy in the solutions of the η-differential equations of the INM model. The local energy η's supposed to carry signature of the characteristic properties of nuclei are found to possess the predictive capability. In fact η-systematics reveal new magic numbers in the drip-line regions giving rise to new islands of stability supported by relativistic mean field theoretic calculations. This is a manifestation of a new phenomenon where shell-effect overcomes the instability due to repulsive components of the nucleon-nucleon force broadening the stability peninsula. The two-neutron separation energy-systematics derived from the present mass predictions reveal a general new feature for the existence of islands of inversion in the exotic neutron-rich regions of nuclear landscape, apart from supporting the presently known islands around 31Na and 62Ti. The five global parameters representing the properties of infinite nuclear matter, the surface, the Coulomb and the pairing terms are retained as per our 1999 mass table. The root-mean-square deviation of the present mass-fit to 2198 known masses is 342 keV, while the mean deviation is 1.3 keV, reminiscent of no left-over systematic effects. This is a substantive improvement over our 1999 mass table having rms deviation of 401 keV and mean deviation of 9 keV for 1884 data nuclei.

  11. Phantom energy: dark energy with w <--1 causes a cosmic doomsday.

    PubMed

    Caldwell, Robert R; Kamionkowski, Marc; Weinberg, Nevin N

    2003-08-15

    We explore the consequences that follow if the dark energy is phantom energy, in which the sum of the pressure and energy density is negative. The positive phantom-energy density becomes infinite in finite time, overcoming all other forms of matter, such that the gravitational repulsion rapidly brings our brief epoch of cosmic structure to a close. The phantom energy rips apart the Milky Way, solar system, Earth, and ultimately the molecules, atoms, nuclei, and nucleons of which we are composed, before the death of the Universe in a "big rip."

  12. An Avalanche Diode Electron Detector for Observing NEET

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kishimoto, Shunji

    2004-05-12

    Nuclear excitation by electron transition (NEET) occurs in atomic inner-shell ionization if the nuclear excitation and the electron transition have nearly the same energy and a common multipolarity. We successfully observed the NEET on 197Au and on 193Ir using a silicon avalanche diode electron detector. The detector was used to find internal conversion electrons emitted from excited nuclei in time spectroscopy with a time gate method. Some nuclear resonant levels, including 8.410 keV on 169Tm and 80.577 keV on 166Er, were also observed with the detector.

  13. Phase transitions in dense matter

    NASA Astrophysics Data System (ADS)

    Dexheimer, Veronica; Hempel, Matthias; Iosilevskiy, Igor; Schramm, Stefan

    2017-11-01

    As the density of matter increases, atomic nuclei disintegrate into nucleons and, eventually, the nucleons themselves disintegrate into quarks. The phase transitions (PT's) between these phases can vary from steep first order to smooth crossovers, depending on certain conditions. First-order PT's with more than one globally conserved charge, so-called non-congruent PT's, have characteristic differences compared to congruent PT's. In this conference proceeding we discuss the non-congruence of the quark deconfinement PT at high densities and/or temperatures relevant for heavy-ion collisions, neutron stars, proto-neutron stars, supernova explosions, and compact-star mergers.

  14. Selected spectroscopic results on element 115 decay chains

    DOE PAGES

    Rudolph, D.; Forsberg, U.; Golubev, P.; ...

    2014-08-24

    We observed thirty correlated α-decay chains in an experiment studying the fusion-evaporation reaction 48Ca + 243Am at the GSI Helmholtzzentrum fur Schwerionenforschung. The decay characteristics of the majority of these 30 chains are consistent with previous observations and interpretations of such chains to originate from isotopes of element Z = 115. High-resolution α-photon coincidence spectroscopy in conjunction with comprehensive Monte-Carlo simulations allow to propose excitation schemes of atomic nuclei of the heaviest elements, thereby probing nuclear structure models near the 'Island of Stability' with unprecedented experimental precision.

  15. Neutrino Oscillations and Neutrino Masses

    NASA Astrophysics Data System (ADS)

    Fritzsch, Harald

    In 1914 James Chadwick discovered that energy and momentum were not conserved in the beta decay of atomic nuclei. For the next 16 years this phenomenon was not understood. In 1930 Wolfgang Pauli suggested in a letter to the participants of a conference in Tuebingen, that in the beta decays not only an electron was emitted, but also a neutral particle, which could not be observed. The energy and momentum of this particle would be the observed missing energy and momentum. Enrico Fermi proposed a name for this hypothetical particle: neutrino...

  16. Biological effects of stellar collapse neutrinos

    PubMed

    Collar, J I

    1996-02-05

    Massive stars in their final stages of collapse radiate most of their binding energy in the form of MeV neutrinos. The recoil atoms that they produce in elastic scattering off nuclei in organic tissue create radiation damage which is highly effective in the production of irreparable DNA harm, leading to cellular mutation, neoplasia, and oncogenesis. Using a conventional model of the galaxy and of the collapse mechanism, the periodicity of nearby stellar collapses and the radiation dose are calculated. The possible contribution of this process to the paleontological record of mass extinctions is examined.

  17. First experiment at TASCA towards X-ray fingerprinting of element 115 decay chains

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Forsberg, U.; Golubev, P.; Sarmiento, L. G.

    2012-01-01

    To identify the atomic number of superheavy nuclei produced in 48Ca-induced fusion-evaporation reactions, an experiment aiming at measuring characteristic X-rays is being prepared at GSI, Darmstadt, Germany. The gas-filled separator TASCA will be employed, sending the residues towards the multi-coincidence detector setup TASISpec. Two ionoptical modes relying on differing magnetic polarities of the quadrupole magnets can be used at TASCA. New simulations and experimental tests of transmission and background suppression for these two focusing modes into TASISpec are presented.

  18. Attempts to Manipulate the Decay Time of Radioactive Nuclei

    NASA Astrophysics Data System (ADS)

    Fallin, B.; Grabow, B.; Tornow, W.

    2008-04-01

    It has been known for 20 years that electron screening strongly changes nuclear reaction cross sections at sub-Coulomb charged-particle projectile energies. The screening energy can be increased considerably if the target atoms are implanted in a metallic host and cooled to low temperature (T˜10 K). The large screening in metals derives from the Debye plasma model applied to the quasi-free metallic electrons. If ``time reversed,'' this model implies that the lifetime of radioactive nuclei placed in a metallic host can be manipulated by orders of magnitude. For α and β^+ decay one expects a shorter half-life, while for β^- decay and EC, a longer half-life is expected. The results of prior experiments testing this theory are controversial; about half of the published data confirm an effect, while the other half observe no effect. We will report on our experimental studies using ^64Cu and ^65Zn nuclei produced at TUNL via the ^63Cu(d,p) and ^65Cu(p,n) reactions, respectively. For ^64Cu, we detected the 511 keV annihilation γ rays and for ^65Zn the 1115.5 keV γ rays using HPGe detectors. In both cases we did not observe a half-life change outside experimental uncertainties between measurements at room temperature and those with the samples cooled to T=12 K.

  19. Atomic-scale investigation of nuclear quantum effects of surface water: Experiments and theory

    NASA Astrophysics Data System (ADS)

    Guo, Jing; Li, Xin-Zheng; Peng, Jinbo; Wang, En-Ge; Jiang, Ying

    2017-12-01

    Quantum behaviors of protons in terms of tunneling and zero-point motion have significant effects on the macroscopic properties, structure, and dynamics of water even at room temperature or higher. In spite of tremendous theoretical and experimental efforts, accurate and quantitative description of the nuclear quantum effects (NQEs) is still challenging. The main difficulty lies in that the NQEs are extremely susceptible to the structural inhomogeneity and local environments, especially when interfacial systems are concerned. In this review article, we will highlight the recent advances of scanning tunneling microscopy and spectroscopy (STM/S), which allows the access to the quantum degree of freedom of protons both in real and energy space. In addition, we will also introduce recent development of ab initio path-integral molecular dynamics (PIMD) simulations at surfaces/interfaces, in which both the electrons and nuclei are treated as quantum particles in contrast to traditional ab initio molecular dynamics (MD). Then we will discuss how the combination of STM/S and PIMD are used to directly visualize the concerted quantum tunneling of protons within the water clusters and quantify the impact of zero-point motion on the strength of a single hydrogen bond (H bond) at a water/solid interface. Those results may open up the new possibility of exploring the exotic quantum states of light nuclei at surfaces, as well as the quantum coupling between the electrons and nuclei.

  20. Implications of supernova remnant origin model of galactic cosmic rays on gamma rays from young supernova remnants

    NASA Astrophysics Data System (ADS)

    Banik, Prabir; Bhadra, Arunava

    2017-06-01

    It is widely believed that Galactic cosmic rays are originated in supernova remnants (SNRs), where they are accelerated by a diffusive shock acceleration (DSA) process in supernova blast waves driven by expanding SNRs. In recent theoretical developments of the DSA theory in SNRs, protons are expected to accelerate in SNRs at least up to the knee energy. If SNRs are the true generators of cosmic rays, they should accelerate not only protons but also heavier nuclei with the right proportions, and the maximum energy of the heavier nuclei should be the atomic number (Z ) times the mass of the proton. In this work, we investigate the implications of the acceleration of heavier nuclei in SNRs on energetic gamma rays produced in the hadronic interaction of cosmic rays with ambient matter. Our findings suggest that the energy conversion efficiency has to be nearly double for the mixed cosmic ray composition compared to that of pure protons to explain observations. In addition, the gamma-ray flux above a few tens of TeV would be significantly higher if cosmic ray particles could attain energies Z times the knee energy in lieu of 200 TeV, as suggested earlier for nonamplified magnetic fields. The two stated maximum energy paradigms will be discriminated in the future by upcoming gamma-ray experiments like the Cherenkov telescope array (CTA).

  1. β-decay spectroscopy of r-process nuclei with N = 126 at KISS

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hirayama, Y.; Watanabe, Y. X.; Imai, N.

    2014-05-02

    The β-decay properties of nuclei with N = 126, which are believed to act as progenitors in the rapid neutron capture (r-) process path forming the third peak (A ∼ 195) in the observed r-abundance element distribution, are considered critical for understanding the production of heavy elements such as gold and platinum at astrophysical sites. We have constructed the KEK Isotope Separation System (KISS), which consists of a gas cell based laser ion source (atomic number selection) and an isotope separation on-line (ISOL) (mass number selection), to produce pure low-energy beams of neutron-rich isotopes around N = 126 and tomore » study their β-decay properties, which are also of interest for astrophysics. The isotopes of interest will be produced by multi-nucleon transfer reactions in heavy ion collisions (e.g. {sup 136}Xe projectile on {sup 198}Pt target). KISS will allow us to study unknown isotopes produced in weak reaction channels under low background conditions. We successfully extracted the stable {sup 56}Fe beam from KISS at the last commissioning on-line experiment with the extraction efficiency of 0.25% and beam purity of more than 98%. We can access the nuclei with N = 126 and measure their half-lives using the KISS in the case of the extraction efficiency of 0.1%.« less

  2. Three-level mixing model for nuclear chiral rotation: Role of the planar component

    NASA Astrophysics Data System (ADS)

    Chen, Q. B.; Starosta, K.; Koike, T.

    2018-04-01

    Three- and two-level mixing models are proposed to understand the doubling of states at the same spin and parity in triaxially deformed atomic nuclei with odd numbers of protons and neutrons. The particle-rotor model for such nuclei is solved using the newly proposed basis which couples angular momenta of two valence nucleons and the rotating triaxial mean field into left-handed |L > , right-handed |R > , and planar |P > configurations. The presence and impact of the planar component is investigated as a function of the total spin for mass A ≈130 nuclei with the valence h11 /2 proton particle, valence h11 /2 neutron hole, and the maximum difference between principal axes allowed by the quadrupole deformation of the mean field. It is concluded that at each spin value the higher energy member of a doublet of states is built on the antisymmetric combination of |L > and |R > and is free of the |P > component, indicating that it is of pure chiral geometry. For the lower energy member of the doublet, the contribution of the |P > component to the eigenfunction first decreases and then increases as a function of the total spin. This trend as well as the energy splitting between the doublet states are both determined by the Hamiltonian matrix elements between the planar (|P > ) and nonplanar (|L > and |R > ) subspaces of the full Hilbert space.

  3. Issues and Consequences of Atomic Oxygen Undercutting of Protected Polymers in Low Earth Orbit

    NASA Technical Reports Server (NTRS)

    Banks, Bruce A.; Snyder, Aaron; Miller, Sharon K.; Demko, Rikako

    2002-01-01

    Hydrocarbon based polymers that are exposed to atomic oxygen in low Earth orbit are slowly oxidized which results in recession of their surface. Atomic oxygen protective coatings have been developed which are both durable to atomic oxygen and effective in protecting underlying polymers. However, scratches, pin window defects, polymer surface roughness and protective coating layer configuration can result in erosion and potential failure of protected thin polymer films even though the coatings are themselves atomic oxygen durable. This paper will present issues that cause protective coatings to become ineffective in some cases yet effective in others due to the details of their specific application. Observed in-space examples of failed and successfully protected materials using identical protective thin films will be discussed and analyzed. Proposed approaches to prevent the failures that have been observed will also be presented.

  4. 75 FR 24755 - DTE ENERGY; Enrico Fermi Atomic Power Plant Unit 1; Exemption From Certain Low-Level Waste...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2010-05-05

    ... NUCLEAR REGULATORY COMMISSION [Docket No. 50-16; NRC-2009-0073] DTE ENERGY; Enrico Fermi Atomic... License No. DPR-9 issued for Enrico Fermi Atomic Power Plant, Unit 1 (Fermi-1), located in Monroe County... undue hazard to life or property. There are no provisions in the Atomic Energy Act (or in any other...

  5. Ultra-sensitive atomic magnetometer for studying magnetization fields produced by hyperpolarized helium-3

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Zou, Sheng; Zhang, Hong; Fang, Jian-cheng, E-mail: fangjiancheng@buaa.edu.cn

    2016-04-14

    An ingenious approach to acquire the absolute magnetization fields produced by polarized atoms has been presented in this paper. The method was based on detection of spin precession signal of the hyperpolarized helium-3 with ultra-sensitive atomic magnetometer of potassium by referring to time-domain analysis. At first, dynamic responses of the mixed spin ensembles in the presence of variant external magnetic fields have been analyzed by referring to the Bloch equation. Subsequently, the relevant equipment was established to achieve the functions of hyperpolarizing helium-3 and detecting the precession of spin-polarized noble gas. By analyzing the transient response of the magnetometer inmore » time domain, we obtained the relevant damping ratio and natural frequency. When the value of damping ratio reached the maximum value of 0.0917, the combined atomic magnetometer was in equilibrium. We draw a conclusion from the steady response: the magnetization fields of the polarized electrons and the hyperpolarized nuclei were corresponding 16.12 nT and 90.74 nT. Under this situation, the nuclear magnetization field could offset disturbing magnetic fields perpendicular to the orientation of the electronic polarization, and it preserved the electronic spin staying in a stable axis. Therefore, the combined magnetometer was particularly attractive for inertial measurements.« less

  6. Gamow-Teller response in the configuration space of a density-functional-theory-rooted no-core configuration-interaction model

    NASA Astrophysics Data System (ADS)

    Konieczka, M.; Kortelainen, M.; Satuła, W.

    2018-03-01

    Background: The atomic nucleus is a unique laboratory in which to study fundamental aspects of the electroweak interaction. This includes a question concerning in medium renormalization of the axial-vector current, which still lacks satisfactory explanation. Study of spin-isospin or Gamow-Teller (GT) response may provide valuable information on both the quenching of the axial-vector coupling constant as well as on nuclear structure and nuclear astrophysics. Purpose: We have performed a seminal calculation of the GT response by using the no-core configuration-interaction approach rooted in multireference density functional theory (DFT-NCCI). The model treats properly isospin and rotational symmetries and can be applied to calculate both the nuclear spectra and transition rates in atomic nuclei, irrespectively of their mass and particle-number parity. Methods: The DFT-NCCI calculation proceeds as follows: First, one builds a configuration space by computing relevant, for a given physical problem, (multi)particle-(multi)hole Slater determinants. Next, one applies the isospin and angular-momentum projections and performs the isospin and K mixing in order to construct a model space composed of linearly dependent states of good angular momentum. Eventually, one mixes the projected states by solving the Hill-Wheeler-Griffin equation. Results: The method is applied to compute the GT strength distribution in selected N ≈Z nuclei including the p -shell 8Li and 8Be nuclei and the s d -shell well-deformed nucleus 24Mg. In order to demonstrate a flexibility of the approach we present also a calculation of the superallowed GT β decay in doubly-magic spherical 100Sn and the low-spin spectrum in 100In. Conclusions: It is demonstrated that the DFT-NCCI model is capable of capturing the GT response satisfactorily well by using a relatively small configuration space, exhausting simultaneously the GT sum rule. The model, due to its flexibility and broad range of applicability, may either serve as a complement or even as an alternative to other theoretical approaches, including the conventional nuclear shell model.

  7. Empirical mass formula with proton-neutron interaction

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Tachibana, T.; Uno, M.; Yamada, S.

    An atomic mass formula consisting of a gross part, and averge even-odd part and an empirical shell part is studied. The gross part is, apart from a small atomic term, taken to be the sum of nucleon rest masses. Coulomb energies and a polynomial in A/sup 1/3/ and chemically bondN-Zchemically bond/A. The shell part includes, in addition to proton and neutron support of nuclear magicities and the cooperative deformation effect. After the first construction of such a formula, refinements have been made in two respects. One is a separate treatment of Z = N odd-odd nuclei suggested by a quartetmore » model, and the other is an improvement of the proton neutron interaction term. By these refinements the root-mean-square deviation of calculated masses from the 1986 Audi-Wapstra masses has been reduced from 538 keV to 460 keV.« less

  8. Communication: Nuclear quadrupole moment-induced Cotton-Mouton effect in noble gas atoms

    NASA Astrophysics Data System (ADS)

    Fu, Li-juan; Rizzo, Antonio; Vaara, Juha

    2013-11-01

    New, high-sensitivity and high-resolution spectroscopic and imaging methods may be developed by exploiting nuclear magneto-optic effects. A first-principles electronic structure formulation of nuclear electric quadrupole moment-induced Cotton-Mouton effect (NQCME) is presented for closed-shell atoms. In NQCME, aligned quadrupole moments alter the index of refraction of the medium along with and perpendicular to the direction of nuclear alignment. The roles of basis-set convergence, electron correlation, and relativistic effects are investigated for three quadrupolar noble gas isotopes: 21Ne, 83Kr, and 131Xe. The magnitude of the resulting ellipticities is predicted to be 10-4-10-6 rad/(M cm) for fully spin-polarized nuclei. These should be detectable in the Voigt setup. Particularly interesting is the case of 131Xe, in which a high degree of spin polarization can be achieved via spin-exchange optical hyperpolarization.

  9. Calculation of background effects on the VESUVIO eV neutron spectrometer

    NASA Astrophysics Data System (ADS)

    Mayers, J.

    2011-01-01

    The VESUVIO spectrometer at the ISIS pulsed neutron source measures the momentum distribution n(p) of atoms by 'neutron Compton scattering' (NCS). Measurements of n(p) provide a unique window into the quantum behaviour of atomic nuclei in condensed matter systems. The VESUVIO 6Li-doped neutron detectors at forward scattering angles were replaced in February 2008 by yttrium aluminium perovskite (YAP)-doped γ-ray detectors. This paper compares the performance of the two detection systems. It is shown that the YAP detectors provide a much superior resolution and general performance, but suffer from a sample-dependent gamma background. This report details how this background can be calculated and data corrected. Calculation is compared with data for two different instrument geometries. Corrected and uncorrected data are also compared for the current instrument geometry. Some indications of how the gamma background can be reduced are also given.

  10. Davisson-Germer Prize in Atomic or Surface Physics: The COLTRIMS multi-particle imaging technique-new Insight into the World of Correlation

    NASA Astrophysics Data System (ADS)

    Schmidt-Bocking, Horst

    2008-05-01

    The correlated many-particle dynamics in Coulombic systems, which is one of the unsolved fundamental problems in AMO-physics, can now be experimentally approached with so far unprecedented completeness and precision. The recent development of the COLTRIMS technique (COLd Target Recoil Ion Momentum Spectroscopy) provides a coincident multi-fragment imaging technique for eV and sub-eV fragment detection. In its completeness it is as powerful as the bubble chamber in high energy physics. In recent benchmark experiments quasi snapshots (duration as short as an atto-sec) of the correlated dynamics between electrons and nuclei has been made for atomic and molecular objects. This new imaging technique has opened a powerful observation window into the hidden world of many-particle dynamics. Recent multiple-ionization studies will be presented and the observation of correlated electron pairs will be discussed.

  11. NMR Knight shifts and the electronic properties of Rb{sub 8}Na{sub 16}Si{sub 136} clathrate

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Latturner, Susan; Iversen, Bo B.; Sepa, Jelena

    2001-03-15

    A silicon framework clathrate type-II compound was synthesized with rubidium and sodium atoms in cages. A single crystal of this material was characterized by both conventional and synchrotron x-ray diffraction; the structure belongs to the cubic space group Fd-3m, with a cell edge of 14.738(1) Aa. The alkali metals are ordered in the structure, with the small cages containing sodium, and the large cages containing rubidium. Variable temperature magic-angle-spinning NMR of all three nuclei show large Knight shifts with a strong temperature dependence, unlike conventional metals. The low conductivity (200 S/cm) and high paramagnetic susceptibility (5x10{sup -6}emu/g) indicate that asmore » the temperature is lowered, the electrons become more localized on the alkali atoms, resulting in properties consistent with a correlated narrow band metal system.« less

  12. 10 CFR 1017.30 - Criminal penalty.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... INFORMATION Violations § 1017.30 Criminal penalty. Any person who violates section 148 of the Atomic Energy Act or any regulation or order of the Secretary issued under section 148 of the Atomic Energy Act, including these regulations, may be subject to a criminal penalty under section 223 of the Atomic Energy Act...

  13. 10 CFR 1017.30 - Criminal penalty.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... INFORMATION Violations § 1017.30 Criminal penalty. Any person who violates section 148 of the Atomic Energy Act or any regulation or order of the Secretary issued under section 148 of the Atomic Energy Act, including these regulations, may be subject to a criminal penalty under section 223 of the Atomic Energy Act...

  14. 10 CFR 1017.30 - Criminal penalty.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... INFORMATION Violations § 1017.30 Criminal penalty. Any person who violates section 148 of the Atomic Energy Act or any regulation or order of the Secretary issued under section 148 of the Atomic Energy Act, including these regulations, may be subject to a criminal penalty under section 223 of the Atomic Energy Act...

  15. 10 CFR 110.50 - Terms.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... provisions of the Atomic Energy Act and to all applicable rules, regulations, decisions and orders of the... conditions when required by amendments of the Atomic Energy Act or other applicable law, or by other rules, regulations, decisions or orders issued in accordance with the terms of the Atomic Energy Act or other...

  16. 29 CFR 1910.1096 - Ionizing radiation.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... material, as defined in the Atomic Energy Act of 1954, as amended, under a license issued by the Nuclear... material, byproduct material, or special nuclear material, as defined in the Atomic Energy Act of 1954, as... source material, byproduct material, or special nuclear material, as defined in the Atomic Energy Act of...

  17. 29 CFR 1910.1096 - Ionizing radiation.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... material, as defined in the Atomic Energy Act of 1954, as amended, under a license issued by the Nuclear... material, byproduct material, or special nuclear material, as defined in the Atomic Energy Act of 1954, as... source material, byproduct material, or special nuclear material, as defined in the Atomic Energy Act of...

  18. 29 CFR 1910.1096 - Ionizing radiation.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... material, as defined in the Atomic Energy Act of 1954, as amended, under a license issued by the Nuclear... material, byproduct material, or special nuclear material, as defined in the Atomic Energy Act of 1954, as... source material, byproduct material, or special nuclear material, as defined in the Atomic Energy Act of...

  19. Selective excitation enables assignment of proton resonances and (1)H-(1)H distance measurement in ultrafast magic angle spinning solid state NMR spectroscopy.

    PubMed

    Zhang, Rongchun; Ramamoorthy, Ayyalusamy

    2015-07-21

    Remarkable developments in ultrafast magic angle spinning (MAS) solid-state NMR spectroscopy enabled proton-based high-resolution multidimensional experiments on solids. To fully utilize the benefits rendered by proton-based ultrafast MAS experiments, assignment of (1)H resonances becomes absolutely necessary. Herein, we propose an approach to identify different proton peaks by using dipolar-coupled heteronuclei such as (13)C or (15)N. In this method, after the initial preparation of proton magnetization and cross-polarization to (13)C nuclei, transverse magnetization of desired (13)C nuclei is selectively prepared by using DANTE (Delays Alternating with Nutations for Tailored Excitation) sequence and then, it is transferred to bonded protons with a short-contact-time cross polarization. Our experimental results demonstrate that protons bonded to specific (13)C atoms can be identified and overlapping proton peaks can also be assigned. In contrast to the regular 2D HETCOR experiment, only a few 1D experiments are required for the complete assignment of peaks in the proton spectrum. Furthermore, the finite-pulse radio frequency driven recoupling sequence could be incorporated right after the selection of specific proton signals to monitor the intensity buildup for other proton signals. This enables the extraction of (1)H-(1)H distances between different pairs of protons. Therefore, we believe that the proposed method will greatly aid in fast assignment of peaks in proton spectra and will be useful in the development of proton-based multi-dimensional solid-state NMR experiments to study atomic-level resolution structure and dynamics of solids.

  20. Impact of physical confinement on nuclei geometry and cell division dynamics in 3D spheroids.

    PubMed

    Desmaison, Annaïck; Guillaume, Ludivine; Triclin, Sarah; Weiss, Pierre; Ducommun, Bernard; Lobjois, Valérie

    2018-06-08

    Multicellular tumour spheroids are used as a culture model to reproduce the 3D architecture, proliferation gradient and cell interactions of a tumour micro-domain. However, their 3D characterization at the cell scale remains challenging due to size and cell density issues. In this study, we developed a methodology based on 3D light sheet fluorescence microscopy (LSFM) image analysis and convex hull calculation that allows characterizing the 3D shape and orientation of cell nuclei relative to the spheroid surface. By using this technique and optically cleared spheroids, we found that in freely growing spheroids, nuclei display an elongated shape and are preferentially oriented parallel to the spheroid surface. This geometry is lost when spheroids are grown in conditions of physical confinement. Live 3D LSFM analysis of cell division revealed that confined growth also altered the preferential cell division axis orientation parallel to the spheroid surface and induced prometaphase delay. These results provide key information and parameters that help understanding the impact of physical confinement on cell proliferation within tumour micro-domains.

  1. On-line compensation for perturbations of a reaching movement is cerebellar dependent: support for the task dependency hypothesis.

    PubMed

    Shimansky, Yury; Wang, Jian-Jun; Bauer, Richard A; Bracha, Vlastislav; Bloedel, James R

    2004-03-01

    Although the cerebellum has been shown to be critical for the acquisition and retention of adaptive modifications in certain reflex behaviors, this structure's role in the learning of motor skills required to execute complex voluntary goal-directed movements still is unclear. This study explores this issue by analyzing the effects of inactivating the interposed and dentate cerebellar nuclei on the adaptation required to compensate for an external elastic load applied during a reaching movement. We show that cats with these nuclei inactivated can adapt to predictable perturbations of the forelimb during a goal-directed reach by including a compensatory component in the motor plan prior to movement initiation. In contrast, when comparable compensatory modifications must be triggered on-line because the perturbations are applied in randomized trials (i.e., unpredictably), such adaptive responses cannot be executed or reacquired after the interposed and dentate nuclei are inactivated. These findings provide the first demonstration of the condition-dependent nature of the cerebellum's contribution to the learning of a specific volitional task.

  2. BOOK REVIEW: The Harvest of a Century: Discoveries of Modern Physics in 100 Episodes

    NASA Astrophysics Data System (ADS)

    Pisut, Ján

    2009-07-01

    The subtitle of the book is exact: the book presents an impression of the development of physics between 1895 (Röntgen's x-rays) and 2001 (Neutrinos have mass). Each episode describes a particular discovery in about five pages in an easily readable style. More demanding explanations are presented in inserted boxes. A nice feature of the book is that many episodes contain the original drawing of the scheme of the experiment, so that the reader can see how it really happened. For most of the past century, certainly for its first half, physics was the leading science and brought fundamental discoveries in the structure of matter, including the structure of nuclei and particles, and the structure of space-time. Most of the episodes in the book concern these two general fields. Among the episodes are the discoveries of radioactivity, the atomic nucleus, the structure of the atom, quantum mechanics, the theory of relativity, accelerators, superconductivity, superfluidity, nuclear reactions in stars, and also transistors, masers, lasers, black-body radiation of the Universe and Bose-Einstein condensation of atoms in traps amongst others. The author is to be congratulated for the selection of the 100 episodes, as it must have been a difficult task. The discovery of the structure of haemoglobin in Bragg's laboratory received only two lines, and there is no mention of the explanation of the chemical bond in hydrogen molecules or on the construction of fantastic medical instruments based on discoveries in physics. Perhaps there is scope in the future for another 100 episodes of discoveries in multidisciplinary fields where physics has played an essential role. Even some discoveries in pure physics could not be included, for instance, super-heavy nuclei. I would like to recommend this book to all those who like the history of physics and admire its achievements in the past century. In particular, I would also like to recommend it to teachers of introductory courses in atomic and nuclear physics at universities. The schemes of classical experiments in some of the episodes can be used to show how it really was, and material on the physicists themselves can be used for motivating students. Some of the episodes may also be useful for high-school students.

  3. Dynamics of multiple nuclei in Ashbya gossypii hyphae depend on the control of cytoplasmic microtubules length by Bik1, Kip2, Kip3, and not on a capture/shrinkage mechanism.

    PubMed

    Grava, Sandrine; Philippsen, Peter

    2010-11-01

    Ashbya gossypii has a budding yeast-like genome but grows exclusively as multinucleated hyphae. In contrast to budding yeast where positioning of nuclei at the bud neck is a major function of cytoplasmic microtubules (cMTs), A. gossypii nuclei are constantly in motion and positioning is not an issue. To investigate the role of cMTs in nuclear oscillation and bypassing, we constructed mutants potentially affecting cMT lengths. Hyphae lacking the plus (+)end marker Bik1 or the kinesin Kip2 cannot polymerize long cMTs and lose wild-type nuclear movements. Interestingly, hyphae lacking the kinesin Kip3 display longer cMTs concomitant with increased nuclear oscillation and bypassing. Polymerization and depolymerization rates of cMTs are 3 times higher in A. gossypii than in budding yeast and cMT catastrophes are rare. Growing cMTs slide along the hyphal cortex and exert pulling forces on nuclei. Surprisingly, a capture/shrinkage mechanism seems to be absent in A. gossypii. cMTs reaching a hyphal tip do not shrink, and cMT +ends accumulate in hyphal tips. Thus, differences in cMT dynamics and length control between budding yeast and A. gossypii are key elements in the adaptation of the cMT cytoskeleton to much longer cells and much higher degrees of nuclear mobilities.

  4. Kinetic Atom.

    ERIC Educational Resources Information Center

    Wilson, David B.

    1981-01-01

    Surveys the research of scientists like Joule, Kelvin, Maxwell, Clausius, and Boltzmann as it comments on the basic conceptual issues involved in the development of a more precise kinetic theory and the idea of a kinetic atom. (Author/SK)

  5. O-atom degradation mechanisms of materials

    NASA Technical Reports Server (NTRS)

    Coulter, Daniel R.; Liang, Ranty H.; Chung, Shirley Y.; Smith, Keri Oda; Gupta, Amitava

    1987-01-01

    The low Earth orbit environment is described and the critical issues relating to oxygen atom degradation are discussed. Some analytic techniques for studying the problem and preliminary results on the underlying degradation mechanisms are presented.

  6. Atomic Oxygen Task

    NASA Technical Reports Server (NTRS)

    Hadaway, James B.

    1997-01-01

    This report details work performed by the Center for Applied Optics (CAO) at the University of Alabama in Huntsville (UAH) on the contract entitled 'Atomic Oxygen Task' for NASA's Marshall Space Flight Center (contract NAS8-38609, Delivery Order 109, modification number 1). Atomic oxygen effects on exposed materials remain a critical concern in designing spacecraft to withstand exposure in the Low Earth Orbit (LEO) environment. The basic objective of atomic oxygen research in NASA's Materials & Processes (M&P) Laboratory is to provide the solutions to material problems facing present and future space missions. The objective of this work was to provide the necessary research for the design of specialized experimental test configurations and development of techniques for evaluating in-situ space environmental effects, including the effects of atomic oxygen and electromagnetic radiation on candidate materials. Specific tasks were performed to address materials issues concerning accelerated environmental testing as well as specifically addressing materials issues of particular concern for LDEF analysis and Space Station materials selection.

  7. Experiment S009: Nuclear Emulsion

    NASA Technical Reports Server (NTRS)

    Odell, F. W.; Shapiro, M. M.; Silberberg, R.; Stiller, B.; Tsao, C. H.; Durgaprasad, N.; Fichtel, C. E.; Guss, D. E.; Reames, D. V.

    1971-01-01

    The first exposure on a spacecraft of a nuclear emulsion apparatus designed to collect 1000 high quality tracks of heavy nuclei under a negligible thickness of matter (0.07 g/sq cm) is described. The cosmic ray detector consisted of a stack of nuclear emulsions that were designed to register at least 400 heavy nuclei tracks for each 10 hours of useful exposure. The spacecraft had to be oriented in a heads-up attitude during the 10-hour period to eliminate atmospheric albedo particles. The results are as follows: (1) a definite odd-even effect, with low abundances for elements of atomic number 7, 9, and 11; (2) a ratio O/C approximately 0.9; (3) Ne/C, Mg/C, and Si/C ratios between 0.2 and 0.3; (4) an abundance gap in the region 15 less than or equal to Z less than or equal to 19; and (5) a ratio (20 less than or equal to Z less than or equal to 28)/C 0.2, with a large concentration at Z = 26. These results are indicative that successful exposures of nuclear emulsions were obtained on the Gemini 11 mission.

  8. On Complex Nuclei Energetics in LENR

    NASA Astrophysics Data System (ADS)

    Miley, George H.; Hora, Heinz

    2005-03-01

    Swimming Electron Layer (SEL) theory plus fission of ``complex nuclei'' were proposed earlier to explain reaction products observed in electrolysis with multi-layer thin-film metallic electrodesootnotetext1.G.H. Miley, and J.A. Patterson, J. New Energy, Vol. 1, pp.11-15, (1996).. SEL was then extended to treat gas-diffusion driven transmutation experimentsootnotetextG. H. Miley and H. Hora, ``Nuclear Reactions in Solids,'' APS DNP Mtg., East Lansing, MI, Oct (2002).. It is also consistent with measured charged-particle emission during thin-film electrolysis and x-ray emission during plasma bombardment experimentsootnotetextA. Karabut, ``X-ray emission in high-current glow discharge,'' Proc., ICCF-9, Beijing China, May (2002).. The binding energy per complex nucleon can be estimated by an energy balance combined with identification of products for each complex e.g. complexes of A 39 have ˜ 0.05 MeV/Nucleon, etc, in thin film electrolysis. Energies in gas diffusion experiments are lower due to the reduced trap site potential at the multi-atom surface. In the case of x-ray emission, complexes involve subsurface defect center traps, giving only a few keV/Nucleon, consistent with experiments^3.

  9. Transfer reactions induced by lithium ions

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Ogloblin, A.A.

    The review deals with nuclear reactions induced by /sup 6/Li and /sup 7/ Li io ns having energies between 10 and 30 MeV. Due to the cluster structure of / sup 6/Li (/sup 6/Li= alpha +d) and /sup 7/Li (/sup 7/Li= alpha +t) and the low bindi ng energy of these nuclei, one of the clustcr is directly transferred in (/ sup 6/Li, d), (/sup 7/Li, t) (/sup 6/Li alpha ) and (/sup 7/Li, alpha ) reactions, i.e., the alpha p article, the deuteron, or the triton is directly transferred. Particular attention is paid to the (/sup 6/Li, d) andmore » (/sup 7/Li, t) reactions, in which the cluster-transfe r mechanism (alpha-particle transfer) appear in ita purest fomn. These reactions can be used to study the alpha- particle or quartet states of light nuclei, which are difficult or impossible to excite in any other way. The present state of the theory of multinucleon transfcr reactions is considered and the application of the theory to thc analysis of reactions induced by lithium atoms is discussed. (auth)« less

  10. Pressure dependence of backbone chemical shifts in the model peptides Ac-Gly-Gly-Xxx-Ala-NH2.

    PubMed

    Erlach, Markus Beck; Koehler, Joerg; Crusca, Edson; Kremer, Werner; Munte, Claudia E; Kalbitzer, Hans Robert

    2016-06-01

    For a better understanding of nuclear magnetic resonance (NMR) detected pressure responses of folded as well as unstructured proteins the availability of data from well-defined model systems are indispensable. In this work we report the pressure dependence of chemical shifts of the backbone atoms (1)H(α), (13)C(α) and (13)C' in the protected tetrapeptides Ac-Gly-Gly-Xxx-Ala-NH2 (Xxx one of the 20 canonical amino acids). Contrary to expectation the chemical shifts of these nuclei have a nonlinear dependence on pressure in the range from 0.1 to 200 MPa. The polynomial pressure coefficients B 1 and B 2 are dependent on the type of amino acid studied. The coefficients of a given nucleus show significant linear correlations suggesting that the NMR observable pressure effects in the different amino acids have at least partly the same physical cause. In line with this observation the magnitude of the second order coefficients of nuclei being direct neighbors in the chemical structure are also weakly correlated.

  11. Half-life measurements of isomeric states populated in projectile fragmentation

    NASA Astrophysics Data System (ADS)

    Bowry, M.; Podolyák, Zs.; Kurcewicz, J.; Pietri, S.; Bunce, M.; Regan, P. H.; Farinon, F.; Geissel, H.; Nociforo, C.; Prochazka, A.; Weick, H.; Allegro, P.; Benlliure, J.; Benzoni, G.; Boutachkov, P.; Gerl, J.; Gorska, M.; Gottardo, A.; Gregor, N.; Janik, R.; Knöbel, R.; Kojouharov, I.; Kubo, T.; Litvinov, Y. A.; Merchan, E.; Mukha, I.; Naqvi, F.; Pfeiffer, B.; Pfützner, M.; Plaß, W.; Pomorski, M.; Riese, B.; Ricciardi, M. V.; Schmidt, K.-H.; Schaffner, H.; Kurz, N.; Denis Bacelar, A. M.; Bruce, A. M.; Farrelly, G. F.; Alkhomashi, N.; Al-Dahan, N.; Scheidenberger, C.; Sitar, B.; Spiller, P.; Stadlmann, J.; Strmen, P.; Sun, B.; Takeda, H.; Tanihata, I.; Terashima, S.; Valiente Dobon, J. J.; Winfield, J. S.; Wollersheim, H.-J.; Woods, P. J.

    2012-10-01

    The half-lives of excited isomeric states observed in 195Au, 201Tl and 215Rn are reported for the first time. Delayed γ-rays were correlated with nuclei produced in the projectile fragmentation of relativistic 238U ions, unambiguously identified in terms of their atomic number (Z) and mass-to-charge ratio (A/Q) after traversing an in-flight separator. The observation of a long-lived isomeric state in 195Au with t1/2 = 16-4+8 μs is presented. Two shorter-lived isomeric states were detected in 201Tl and 215Rn with t1/2 = 95-21+39 and 57-12+21 ns respectively. In total 24 isomeric states were identified in different nuclei from Pt to Rn (A ˜ 200) during the current study, the majority of which were previously reported. The wealth of spectroscopic data provides the opportunity to determine the isomeric ratios over a wide range of Z, A and angular momentum (I ħ) of the reaction products. In particular, high-spin states with I ≳ 18 ħ provide a robust test of theoretical models of fragmentation.

  12. Does the Iron K and Alpha: Line of Active Galactic Nuclei Arise from the Cerenkov Line-like Radiation?

    NASA Technical Reports Server (NTRS)

    You, J. H.; Liu, D. B.; Chen, W. P.; Chen, L.; Zhang, S. N.

    2003-01-01

    When thermal relativistic electrons with isotropic distribution of velocities move in a gas region or impinge upon the surface of a cloud that consists of a dense gas or doped dusts, the Cerenkov effect produces peculiar atomic or ionic emission lines, which is known as the Cerenkov line - like radiation. This newly recognized emission mechanism may find wide applications in high-energy astrophysics. In this paper we tentatively adopt this new line emission mechanism to discuss the origin of the iron Kα feature of active galactic nuclei (AGNs). The motivation of this research is to attempt a solution to a problem encountered by the "disk fluorescence line" model, i.e. , the lack of temporal response of the observed iron Kα line flux to the changes of the X-ray continuum flux. If the Cerenkov line emission is indeed responsible significant ly for the iron Kα feature, the conventional scenario around the central supermassive black holes of AGNs would need to be modified to accomodate more energetic, more violent, and much denser environments than previously thought.

  13. Universal odd-even staggering in isotopic fragmentation and spallation cross sections of neutron-rich fragments

    NASA Astrophysics Data System (ADS)

    Mei, B.; Tu, X. L.; Wang, M.

    2018-04-01

    An evident odd-even staggering (OES) in fragment cross sections has been experimentally observed in many fragmentation and spallation reactions. However, quantitative comparisons of this OES effect in different reaction systems are still scarce for neutron-rich nuclei near the neutron drip line. By employing a third-order difference formula, the magnitudes of this OES in extensive experimental cross sections are systematically investigated for many neutron-rich nuclei with (N -Z ) from 1 to 23 over a broad range of atomic numbers (Z ≈3 -50 ). A comparison of these magnitude values extracted from fragment cross sections measured in different fragmentation and spallation reactions with a large variety of projectile-target combinations over a wide energy range reveals that the OES magnitude is almost independent of the projectile-target combinations and the projectile energy. The weighted average of these OES magnitudes derived from cross sections accurately measured in different reaction systems is adopted as the evaluation value of the OES magnitude. These evaluated OES magnitudes are recommended to be used in fragmentation and spallation models to improve their predictions for fragment cross sections.

  14. Measurement of Activation Cross Sections Producing Short-Lived Nuclei with Pulsed Neutron Beam

    NASA Astrophysics Data System (ADS)

    Shimizu, Toshiaki; Arakita, Kazumasa; Miyazaki, Itaru; Shibata, Michihiro; Kawade, Kiyoshi; Hori, Jun-ichi; Ochiai, Kentaro; Nishitani, Takeo

    2005-05-01

    Activation cross sections for the (n, n') reaction were measured by means of the activation method at the neutron energies of 3.1 and 2.54 MeV by using a pulsed neutron beam. Target nuclei were 79Br, 90Zr, 197Au, and 207Pb, whose half-lives were between 0.8 and 8 s. The cross section for the 90Zr (n, n') 90mZr reaction was obtained for the first time in this energy range. The d-D neutrons were generated by bombarding a deuterated titanium target with a 350-keV d+ beam at the 80-degree beam line of the Fusion Neutronics Source at the Japan Atomic Energy Research Institute. In order to obtain reliable activation cross sections, careful attention was paid to correct the efficiency for a volume source, and the self-absorption of gamma rays in an irradiated sample. The systematics of the (n, n') reaction at the neutron energy of 3.1 MeV, which could be predicted within an accuracy of 50%, was proposed on the basis of our data.

  15. 26Al Production in the Early Solar Nebula by Neutral High-Energy Plasma Winds

    NASA Astrophysics Data System (ADS)

    Spergel, M. S.

    1995-09-01

    In the light of recent observations, I believe that the sources for the presence of ^26Al within the solar nebula must be reconsidered [2,3]. Recent low observational estimates of the probability of encounters between mass-losing evolved stars and molecular clouds [4] for the production of ^26Al and the observed low production [5] of 26 Al from AGB (Asymptotic Giant Branch stars) along with the predicted low abundance of cosmic ray induced local production [6] in the early solar nebula all support continued investigation for additional sources of the solar nebula ^26Al presence. It is suggested based on the presences of new cross section data [7], that an important source of this ^26Al presence might be from enhanced interactions from the collisions of the local "T. Tauri" like plasma winds with the atomic and molecular Early Solar Nebula (ESN). Interactions like ^26Mg (p,n) ^26Al in this "neutral" electrical setting may provide the needed selective production. The ESN provides an environment where plasma winds can lead to such nucleosynthesis. Stellar winds of 300-700 km/s (about 3x10^7 K) are seen to T. Tauri like stars, presumed precursor to solar like stars, and also within the Solar heliosphere [8.9]. These winds provide the source of Solar High Energy Particles which can interact with such in situ targets such as ^26Mg to produce the ^26Al. The presence of the atomic and molecular environments, will enhance [10] nucleosynthesis over that seen in scattering of protons off bare nuclei. Such enhancement has been recently observed in low energy scattering on electrically shield targets [7]. There it was also suggested that in stellar convective zones, electron clouds of the plasma shield may also shield bare target nuclei. Measured values of low energy proton scattered on atomic and molecular targets indicated [7] that fusion cross sections are enlarged and elastic cross sections are reduced, therefore simple extrapolation of accelerator data can lead to an underestimate in the relevant excitation cross sections in lower energy proton induced production. Enhanced production in the ESN will be from the shielded atomic or molecular nuclei with the production increased by the product of this enhanced proton nucleosynthesis and the presence of the higher proton intensities for the lower energy particles available in the solar wind. References: [1] Supported under NIH-MARC grant #443789. [2] Clayton D. D. et al. (1977) Astrophys. J., 214, 300-315. [3] Clayton D. D. (1994) Nature, 368, 222-224. [4] Kastner J. H. and Myers P. C. (1994) Astrophys. J., 421, 605-614. [5] Prantzos N. (1993) Astrophys. J. Lett., 405, L55-L58. [6] Spergel M. S. (1995) Astrophys. Space Sci., 223, 187. [7] Castellani V. et al., The fate of Li and Be in stars and in the Laboratory, INFNFE-04-95 (preprint). [8] Simpson J. A. et al. (1995) Science, 268, 1019-1023. [9] Keppler E. et al. (1995) Science, 268, 1013-1016. [10] Rolfs C. E. and Rodney W. S. (1988) Cauldrons in the Cosmos (Nuclear Astrophysics), 165-168, Univ. of California.

  16. Mass analyzer ``MASHA'' high temperature target and plasma ion source

    NASA Astrophysics Data System (ADS)

    Semchenkov, A. G.; Rassadov, D. N.; Bekhterev, V. V.; Bystrov, V. A.; Chizov, A. Yu.; Dmitriev, S. N.; Efremov, A. A.; Guljaev, A. V.; Kozulin, E. M.; Oganessian, Yu. Ts.; Starodub, G. Ya.; Voskresensky, V. M.; Bogomolov, S. L.; Paschenko, S. V.; Zelenak, A.; Tikhonov, V. I.

    2004-05-01

    A new separator and mass analyzer of super heavy atoms (MASHA) has been created at the FLNR JINR Dubna to separate and measure masses of nuclei and molecules with precision better than 10-3. First experiments with the FEBIAD plasma ion source have been done and give an efficiency of ionization of up to 20% for Kr with a low flow test leak (6 particle μA). We suppose a magnetic field optimization, using the additional electrode (einzel lens type) in the extracting system, and an improving of the vacuum conditions in order to increase the ion source efficiency.

  17. Intermediate-energy nuclear chemistry workshop

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Butler, G.W.; Giesler, G.C.; Liu, L.C.

    1981-05-01

    This report contains the proceedings of the LAMPF Intermediate-Energy Nuclear Chemistry Workshop held in Los Alamos, New Mexico, June 23-27, 1980. The first two days of the Workshop were devoted to invited review talks highlighting current experimental and theoretical research activities in intermediate-energy nuclear chemistry and physics. Working panels representing major topic areas carried out indepth appraisals of present research and formulated recommendations for future research directions. The major topic areas were Pion-Nucleus Reactions, Nucleon-Nucleus Reactions and Nuclei Far from Stability, Mesonic Atoms, Exotic Interactions, New Theoretical Approaches, and New Experimental Techniques and New Nuclear Chemistry Facilities.

  18. A theoretical NMR study of selected benzazoles: Comparison of GIPAW and GIAO-PCM (DMSO) calculations.

    PubMed

    Marín-Luna, Marta; Alkorta, Ibon; Elguero, José

    2018-03-01

    This paper compares the absolute shieldings obtained by gauge-including-projected-augmented-wave (GIPAW) to those obtained by gauge-invariant atomic orbital/Becke, 3-parameter, Lee-Yang-Parr (GIAO/B3LYP)/6-311++G(d,p)-polarizable continuum model (PCM, dimethyl sulfoxide) for nine benzazoles (benzimidazoles, indazoles, and benzotriazoles) recorded in the solid-state. Three nuclei were explored, 13 C, 15 N, and 19 F, and the gauge-including-projected-augmented-wave approach only proved better for 15 N MAS NMR. Copyright © 2017 John Wiley & Sons, Ltd.

  19. Ring Around the Black Hole

    NASA Technical Reports Server (NTRS)

    Wanjek, Christopher

    2003-01-01

    Regardless of size, black holes easily acquire accretion disks. Supermassive black holes can feast on the bountiful interstellar gas in galactic nuclei. Small black holes formed from collapsing stars often belong to binary systems in which a bulging companion star can spill some of its gas into the black hole s reach. In the chaotic mess of the accretion disk, atoms collide with one another. Swirling plasma reaches speeds upward of 10% that of light and glows brightly in many wavebands, particularly in X-rays. Gas gets blown back by a wind of radiation from the inner disk. New material enters the disks from different directions.

  20. Multiconfiguration calculations of electronic isotope shift factors in Al i

    NASA Astrophysics Data System (ADS)

    Filippin, Livio; Beerwerth, Randolf; Ekman, Jörgen; Fritzsche, Stephan; Godefroid, Michel; Jönsson, Per

    2016-12-01

    The present work reports results from systematic multiconfiguration Dirac-Hartree-Fock calculations of electronic isotope shift factors for a set of transitions between low-lying levels of neutral aluminium. These electronic quantities together with observed isotope shifts between different pairs of isotopes provide the changes in mean-square charge radii of the atomic nuclei. Two computational approaches are adopted for the estimation of the mass- and field-shift factors. Within these approaches, different models for electron correlation are explored in a systematic way to determine a reliable computational strategy and to estimate theoretical error bars of the isotope shift factors.

  1. Spin accumulation in thin Cs salts on contact with optically polarized Cs vapor

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Ishikawa, Kiyoshi

    2011-09-15

    The spin angular momentum accumulates in the Cs nuclei of salt on contact with optically pumped Cs vapor. The spin polarization in stable chloride as well as dissociative hydride indicates that nuclear dipole interaction works in spin transferring with a lesser role of atom exchange. In the solid film, not only the spin buildup but also the decay of enhanced polarization is faster than the thermal recovery rate for the bulk salt. Eliminating the signal of thick salt, we find that the nuclear spin polarization in the chloride film reaches over 100 times the thermal equilibrium.

  2. The Exploration of Hot Nuclear Matter

    NASA Astrophysics Data System (ADS)

    Jacak, Barbara V.; Müller, Berndt

    2012-07-01

    When nuclear matter is heated beyond 2 trillion degrees, it becomes a strongly coupled plasma of quarks and gluons. Experiments using highly energetic collisions between heavy nuclei have revealed that this new state of matter is a nearly ideal, highly opaque liquid. A description based on string theory and black holes in five dimensions has made the quark-gluon plasma an archetypical strongly coupled quantum system. Open questions about the structure and theory of the quark-gluon plasma are under active investigation. Many of the insights are also relevant to ultracold fermionic atoms and strongly correlated condensed matter.

  3. Extension of the nuclear mass surface for neutron-rich isotopes of argon through iron

    NASA Astrophysics Data System (ADS)

    Meisel, Zachary Paul

    Nuclear mass measurement has maintained an important position in the field of nuclear physics for a little over a century. Nuclear masses provide key evidence of the structural transformation of nuclei away from the valley of beta-stability and are essential input for many simulations of extreme astrophysical environments. However, obtaining these masses is often a challenging endeavor due to the low production cross sections and short half-lives of the exotic nuclei which are of particular interest. To this end, the time-of-flight mass measurement technique has been developed to obtain the masses of several nuclei at once to precisions of 1 part in 105 with virtually no half-life limitation. This dissertation contains a description of the experiment, analysis, and results of the second implementation of the time-of-flight nuclear mass measurement technique at the National Superconducting Cyclotron Laboratory. 18 masses were obtained for neutron-rich isotopes of argon through iron, where the masses of 48Ar, 49Ar, 56Sc, 57Sc, 64Cr, 67Mn, and 69Fe were measured for the first time. These newly obtained masses were applied to outstanding problems in nuclear structure and nuclear astrophysics, resulting in significant scientific advances. The measurement results for 48Ar and 49Ar, which were found to have atomic mass excesses of -22.28(31) MeV and -17.8(1.1) MeV, respectively, provide strong evidence for the closed shell nature of neutron number N = 28 in argon. It follows that argon is therefore the lowest even-Z element exhibiting the N = 28 closed shell. The masses of 64Cr, 67 Mn, and 69Fe, which were found to have atomic mass excesses of -33.48(44) MeV, -34.09(62) MeV, and -39.35(60) MeV, respectively, show signs of nuclear deformation occurring around the N = 40 subshell. In addition, we found 64Cr is substantially less bound than predicted by global mass models that are commonly used in nuclear astrophysics simulations, resulting in a significant reduction in the predicted strength and depth of electron capture heating in the accreted neutron star crust due to the rather abundant A = 64 mass-chain. The reported value for the atomic mass excess of 56Sc, -24.85(59)(+0,-54) MeV, which contains an asymmetric systematic uncertainty due to potential isomeric contamination, results in a smaller than expected odd-even mass staggering in the A = 56 mass chain. Depending on the choice of theoretical models for electron capture transition strengths and energies, this could lead to strong Urca cooling in accreted neutron star crusts, due to the large amount of A = 56 material predicted to be present on the surface of accreted neutron stars.

  4. From atoms to layers: in situ gold cluster growth kinetics during sputter deposition

    NASA Astrophysics Data System (ADS)

    Schwartzkopf, Matthias; Buffet, Adeline; Körstgens, Volker; Metwalli, Ezzeldin; Schlage, Kai; Benecke, Gunthard; Perlich, Jan; Rawolle, Monika; Rothkirch, André; Heidmann, Berit; Herzog, Gerd; Müller-Buschbaum, Peter; Röhlsberger, Ralf; Gehrke, Rainer; Stribeck, Norbert; Roth, Stephan V.

    2013-05-01

    The adjustment of size-dependent catalytic, electrical and optical properties of gold cluster assemblies is a very significant issue in modern applied nanotechnology. We present a real-time investigation of the growth kinetics of gold nanostructures from small nuclei to a complete gold layer during magnetron sputter deposition with high time resolution by means of in situ microbeam grazing incidence small-angle X-ray scattering (μGISAXS). We specify the four-stage growth including their thresholds with sub-monolayer resolution and identify phase transitions monitored in Yoneda intensity as a material-specific characteristic. An innovative and flexible geometrical model enables the extraction of morphological real space parameters, such as cluster size and shape, correlation distance, layer porosity and surface coverage, directly from reciprocal space scattering data. This approach enables a large variety of future investigations of the influence of different process parameters on the thin metal film morphology. Furthermore, our study allows for deducing the wetting behavior of gold cluster films on solid substrates and provides a better understanding of the growth kinetics in general, which is essential for optimization of manufacturing parameters, saving energy and resources.The adjustment of size-dependent catalytic, electrical and optical properties of gold cluster assemblies is a very significant issue in modern applied nanotechnology. We present a real-time investigation of the growth kinetics of gold nanostructures from small nuclei to a complete gold layer during magnetron sputter deposition with high time resolution by means of in situ microbeam grazing incidence small-angle X-ray scattering (μGISAXS). We specify the four-stage growth including their thresholds with sub-monolayer resolution and identify phase transitions monitored in Yoneda intensity as a material-specific characteristic. An innovative and flexible geometrical model enables the extraction of morphological real space parameters, such as cluster size and shape, correlation distance, layer porosity and surface coverage, directly from reciprocal space scattering data. This approach enables a large variety of future investigations of the influence of different process parameters on the thin metal film morphology. Furthermore, our study allows for deducing the wetting behavior of gold cluster films on solid substrates and provides a better understanding of the growth kinetics in general, which is essential for optimization of manufacturing parameters, saving energy and resources. Electronic supplementary information (ESI) available: The full GISAXS image sequence of the experiment, the model-based IsGISAXS-simulation sequence as movie files for comparison and detailed information about sample cleaning, XRR, FESEM, IsGISAXS, comparison μGIWAXS/μGISAXS, and sampling statistics. See DOI: 10.1039/c3nr34216f

  5. Measurement of interaction between antiprotons

    DOE PAGES

    Adamczyk, L.; Adkins, J. K.; Agakishiev, G.; ...

    2015-11-04

    In this paper, one of the primary goals of nuclear physics is to understand the force between nucleons, which is a necessary step for understanding the structure of nuclei and how nuclei interact with each other. Rutherford discovered the atomic nucleus in 1911, and the large body of knowledge about the nuclear force that has since been acquired was derived from studies made on nucleons or nuclei. Although antinuclei up to antihelium-4 have been discovered and their masses measured, little is known directly about the nuclear force between antinucleons. Here, we study antiproton pair correlations among data collected by themore » STAR experiment at the Relativistic Heavy Ion Collider (RHIC), where gold ions are collided with a centre-of-mass energy of 200 gigaelectronvolts per nucleon pair. Antiprotons are abundantly produced in such collisions, thus making it feasible to study details of the antiproton–antiproton interaction. By applying a technique similar to Hanbury Brown and Twiss intensity interferometry, we show that the force between two antiprotons is attractive. In addition, we report two key parameters that characterize the corresponding strong interaction: the scattering length and the effective range of the interaction. Our measured parameters are consistent within errors with the corresponding values for proton–proton interactions. Our results provide direct information on the interaction between two antiprotons, one of the simplest systems of antinucleons, and so are fundamental to understanding the structure of more-complex antinuclei and their properties.« less

  6. Hemispheric aerosol vertical profiles: anthropogenic impacts on optical depth and cloud nuclei.

    PubMed

    Clarke, Antony; Kapustin, Vladimir

    2010-09-17

    Understanding the effect of anthropogenic combustion upon aerosol optical depth (AOD), clouds, and their radiative forcing requires regionally representative aerosol profiles. In this work, we examine more than 1000 vertical profiles from 11 major airborne campaigns in the Pacific hemisphere and confirm that regional enhancements in aerosol light scattering, mass, and number are associated with carbon monoxide from combustion and can exceed values in unperturbed regions by more than one order of magnitude. Related regional increases in a proxy for cloud condensation nuclei (CCN) and AOD imply that direct and indirect aerosol radiative effects are coupled issues linked globally to aged combustion. These profiles constrain the influence of combustion on regional AOD and CCN suitable for challenging climate model performance and informing satellite retrievals.

  7. Electromagnetic Dissociation and Spacecraft Electronics Damage

    NASA Technical Reports Server (NTRS)

    Norbury, John W.

    2016-01-01

    When protons or heavy ions from galactic cosmic rays (GCR) or solar particle events (SPE) interact with target nuclei in spacecraft, there can be two different types of interactions. The more familiar strong nuclear interaction often dominates and is responsible for nuclear fragmentation in either the GCR or SPE projectile nucleus or the spacecraft target nucleus. (Of course, the proton does not break up, except possibly to produce pions or other hadrons.) The less familiar, second type of interaction is due to the very strong electromagnetic fields that exist when two charged nuclei pass very close to each other. This process is called electromagnetic dissociation (EMD) and primarily results in the emission of neutrons, protons and light ions (isotopes of hydrogen and helium). The cross section for particle production is approximately defined as the number of particles produced in nucleus-nucleus collisions or other types of reactions. (There are various kinematic and other factors which multiply the particle number to arrive at the cross section.) Strong, nuclear interactions usually dominate the nuclear reactions of most interest that occur between GCR and target nuclei. However, for heavy nuclei (near Fe and beyond) at high energy the EMD cross section can be much larger than the strong nuclear interaction cross section. This paper poses a question: Are there projectile or target nuclei combinations in the interaction of GCR or SPE where the EMD reaction cross section plays a dominant role? If the answer is affirmative, then EMD mechanisms should be an integral part of codes that are used to predict damage to spacecraft electronics. The question can become more fine-tuned and one can ask about total reaction cross sections as compared to double differential cross sections. These issues will be addressed in the present paper.

  8. Physics Division annual review, 1 April 1980-31 March 1981

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1982-06-01

    Progress in nuclear physics research is reported in the following areas: medium-energy physics (pion reaction mechanisms, high-resolution studies and nuclear structure, and two-nucleon physics with pions and electrons); heavy-ion research at the tandem and superconducting linear accelerator (resonant structure in heavy-ion reactions, fusion cross sections, high angular momentum states in nuclei, and reaction mechanisms and distributions of reaction strengths); charged-particle research; neutron and photonuclear physics; theoretical physics (heavy-ion direct-reaction theory, nuclear shell theory and nuclear structure, nuclear matter and nuclear forces, intermediate-energy physics, microscopic calculations of high-energy collisions of heavy ions, and light ion direct reactions); the superconducting linac; acceleratormore » operations; and GeV electron linac. Progress in atomic and molecular physics research is reported in the following areas: dissociation and other interactions of energetic molecular ions in solid and gaseous targets, beam-foil research and collision dynamics of heavy ions, photoionization- photoelectron research, high-resolution laser rf spectroscopy with atomic and molecular beams, moessbauer effect research, and theoretical atomic physics. Studies on interactions of energetic particles with solids are also described. Publications are listed. (WHK)« less

  9. Geant4 Simulations for the Radon Electric Dipole Moment Search at TRIUMF

    NASA Astrophysics Data System (ADS)

    Rand, Evan; Bangay, Jack; Bianco, Laura; Dunlop, Ryan; Finlay, Paul; Garrett, Paul; Leach, Kyle; Phillips, Andrew; Svensson, Carl; Sumithrarachchi, Chandana; Wong, James

    2010-11-01

    The existence of a permanent electric dipole moment (EDM) requires the violation of time-reversal symmetry (T) or, equivalently, the violation of charge conjugation C and parity P (CP). Although no particle EDM has yet been found, current theories beyond the Standard Model, e.g. multiple-Higgs theories, left-right symmetry, and supersymmetry, predict EDMs within current experimental reach. In fact, present limits on the EDMs of the neutron, electron and ^199Hg atom have significantly reduced the parameter spaces of these models. The measurement of a non-zero EDM would be a direct measurement of the violation of time-reversal symmetry, and would represent a clear signal of new physics beyond the Standard Model. Recent theoretical calculations predict large enhancements in the atomic EDMs for atoms with octupole-deformed nuclei, making odd-A Rn isotopes prime candidates for the EDM search. The Geant4 simulations presented here are essential for the development towards an EDM measurement. They provide an accurate description of γ-ray scattering and backgrounds in the experimental apparatus, and are being used to study the overall sensitivity of the RnEDM experiment at TRIUMF in Vancouver, B.C.

  10. Boosting the Light: X-ray Physics in Confinement

    ScienceCinema

    Rhisberger, Ralf [HASYLAB/ DESY

    2017-12-09

    Remarkable effects are observed if light is confined to dimensions comparable to the wavelength of the light. The lifetime of atomic resonances excited by the radiation is strongly reduced in photonic traps, such as cavities or waveguides. Moreover, one observes an anomalous boost of the intensity scattered from the resonant atoms. These phenomena results from the strong enhancement of the photonic density of states in such geometries. Many of these effects are currently being explored in the regime of vsible light due to their relevance for optical information processing. It is thus appealing to study these phenomena also for much shorter wavelengths. This talk illuminates recent experiments where synchrotron x-rays were trapped in planar waveguides to resonantly excite atomos ([57]Fe nuclei_ embedded in them. In fact, one observes that the radiative decay of these excited atoms is strongly accelerated. The temporal acceleration of the decay goes along with a strong boost of the radiation coherently scattered from the confined atmos. This can be exploited to obtain a high signal-to-noise ratio from tiny quantities of material, leading to manifold applications in the investigation of nanostructured materials. One application is the use of ultrathin probe layers to image the internal structure of magnetic layer systems.

  11. Probing atomic Higgs-like forces at the precision frontier

    NASA Astrophysics Data System (ADS)

    Delaunay, Cédric; Ozeri, Roee; Perez, Gilad; Soreq, Yotam

    2017-11-01

    We propose a novel approach to probe new fundamental interactions using isotope shift spectroscopy in atomic clock transitions. As a concrete toy example we focus on the Higgs boson couplings to the building blocks of matter: the electron and the up and down quarks. We show that the attractive Higgs force between nuclei and their bound electrons, which is poorly constrained, might induce effects that are larger than the current experimental sensitivities. More generically, we discuss how new interactions between the electron and the neutrons, mediated via light new degrees of freedom, may lead to measurable nonlinearities in a King plot comparison between isotope shifts of two different transitions. Given state-of-the-art accuracy in frequency comparison, isotope shifts have the potential to be measured with sub-Hz accuracy, thus potentially enabling the improvement of current limits on new fundamental interactions. A candidate atomic system for this measurement requires two different clock transitions and four zero nuclear spin isotopes. We identify several systems that satisfy this requirement and also briefly discuss existing measurements. We consider the size of the effect related to the Higgs force and the requirements for it to produce an observable signal.

  12. Precision mass measurements of magnesium isotopes and implications for the validity of the isobaric mass multiplet equation

    DOE PAGES

    Brodeur, M.; Kwiatkowski, A. A.; Drozdowski, O. M.; ...

    2017-09-18

    If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the isobaric mass multiplet equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of 29Cl and 30Ar. The atomic mass of 27Mg was found to be within 1.6σ of the value stated in the Atomic Mass Evaluation. The atomic masses of 28,29Mg were measured to be both withinmore » 1σ, while being 7 and 33 times more precise, respectively. Using the 29Mg mass excess and previous measurements of 29Cl, we uncovered a cubic coefficient of d = 28(7)keV, which is the largest known cubic coefficient of the IMME. This departure, however, could also be caused by experimental data with unknown systematic errors. Hence there is a need to confirm the mass excess of 28S and the one-neutron separation energy of 29Cl, which have both come from a single measurement. Lastly, our results were compared with ab initio calculations from the valence-space in-medium similarity renormalization group, resulting in a good agreement.« less

  13. Precision mass measurements of magnesium isotopes and implications for the validity of the isobaric mass multiplet equation

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Brodeur, M.; Kwiatkowski, A. A.; Drozdowski, O. M.

    If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the isobaric mass multiplet equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of 29Cl and 30Ar. The atomic mass of 27Mg was found to be within 1.6σ of the value stated in the Atomic Mass Evaluation. The atomic masses of 28,29Mg were measured to be both withinmore » 1σ, while being 7 and 33 times more precise, respectively. Using the 29Mg mass excess and previous measurements of 29Cl, we uncovered a cubic coefficient of d = 28(7)keV, which is the largest known cubic coefficient of the IMME. This departure, however, could also be caused by experimental data with unknown systematic errors. Hence there is a need to confirm the mass excess of 28S and the one-neutron separation energy of 29Cl, which have both come from a single measurement. Lastly, our results were compared with ab initio calculations from the valence-space in-medium similarity renormalization group, resulting in a good agreement.« less

  14. Proceedings of the NASA Workshop on Atomic Oxygen Effects. [low earth orbital environment

    NASA Technical Reports Server (NTRS)

    Brinza, David E. (Editor)

    1987-01-01

    A workshop was held to address the scientific issues concerning the effects of atomic oxygen on materials in the low Earth orbital (LEO) environment. The program included 18 invited speakers plus contributed posters covering topics such as LEO spaceflight experiments, interaction mechanisms, and atomic oxygen source development. Discussion sessions were also held to organize a test program to evaluate atomic oxygen exposure facilities. The key issues raised in the workshop were: (1) the need to develop a reliable predictive model of the effects of long-term exposure of materials to the LEO environment; (2) the ability of ground-based exposure facilities to provide useful data for development of durable materials; and (3) accurate determination of the composition of the LEO environment. These proceedings include the invited papers, the abstracts for the contributed posters, and an account of the test program discussion sessions.

  15. Plant maintenance and advanced reactors issue, 2008

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Agnihotri, Newal

    The focus of the September-October issue is on plant maintenance and advanced reactors. Major articles/reports in this issue include: Technologies of national importance, by Tsutomu Ohkubo, Japan Atomic Energy Agency, Japan; Modeling and simulation advances brighten future nuclear power, by Hussein Khalil, Argonne National Laboratory, Energy and desalination projects, by Ratan Kumar Sinha, Bhabha Atomic Research Centre, India; A plant with simplified design, by John Higgins, GE Hitachi Nuclear Energy; A forward thinking design, by Ray Ganthner, AREVA; A passively safe design, by Ed Cummins, Westinghouse Electric Company; A market-ready design, by Ken Petrunik, Atomic Energy of Canada Limited, Canada;more » Generation IV Advanced Nuclear Energy Systems, by Jacques Bouchard, French Commissariat a l'Energie Atomique, France, and Ralph Bennett, Idaho National Laboratory; Innovative reactor designs, a report by IAEA, Vienna, Austria; Guidance for new vendors, by John Nakoski, U.S. Nuclear Regulatory Commission; Road map for future energy, by John Cleveland, International Atomic Energy Agency, Vienna, Austria; and, Vermont's largest source of electricity, by Tyler Lamberts, Entergy Nuclear Operations, Inc. The Industry Innovation article is titled Intelligent monitoring technology, by Chris Demars, Exelon Nuclear.« less

  16. NuSTEC1 White Paper: Status and challenges of neutrino-nucleus scattering

    NASA Astrophysics Data System (ADS)

    Alvarez-Ruso, L.; Sajjad Athar, M.; Barbaro, M. B.; Cherdack, D.; Christy, M. E.; Coloma, P.; Donnelly, T. W.; Dytman, S.; de Gouvêa, A.; Hill, R. J.; Huber, P.; Jachowicz, N.; Katori, T.; Kronfeld, A. S.; Mahn, K.; Martini, M.; Morfín, J. G.; Nieves, J.; Perdue, G. N.; Petti, R.; Richards, D. G.; Sánchez, F.; Sato, T.; Sobczyk, J. T.; Zeller, G. P.

    2018-05-01

    The precise measurement of neutrino properties is among the highest priorities in fundamental particle physics, involving many experiments worldwide. Since the experiments rely on the interactions of neutrinos with bound nucleons inside atomic nuclei, the planned advances in the scope and precision of these experiments require a commensurate effort in the understanding and modeling of the hadronic and nuclear physics of these interactions, which is incorporated as a nuclear model in neutrino event generators. This model is essential to every phase of experimental analyses and its theoretical uncertainties play an important role in interpreting every result. In this White Paper we discuss in detail the impact of neutrino-nucleus interactions, especially the nuclear effects, on the measurement of neutrino properties using the determination of oscillation parameters as a central example. After an Executive Summary and a concise Overview of the issues, we explain how the neutrino event generators work, what can be learned from electron-nucleus interactions and how each underlying physics process - from quasi-elastic to deep inelastic scattering - is understood today. We then emphasize how our understanding must improve to meet the demands of future experiments. With every topic we find that the challenges can be met only with the active support and collaboration among specialists in strong interactions and electroweak physics that include theorists and experimentalists from both the nuclear and high energy physics communities.

  17. NuSTEC White Paper: Status and Challenges of Neutrino-Nucleus Scattering

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Alvarez-Ruso, L.; et al.

    The precise measurement of neutrino properties is among the highest priorities in fundamental particle physics, involving many experiments worldwide. Since the experiments rely on the interactions of neutrinos with bound nucleons inside atomic nuclei, the planned advances in the scope and precision of these experiments requires a commensurate effort in the understanding and modeling of the hadronic and nuclear physics of these interactions, which is incorporated as a nuclear model in neutrino event generators. This model is essential to every phase of experimental analyses and its theoretical uncertainties play an important role in interpreting every result. In this White Papermore » we discuss in detail the impact of neutrino-nucleus interactions, especially the nuclear effects, on the measurement of neutrino properties using the determination of oscillation parameters as a central example. After an Executive Summary and a concise Overview of the issues, we explain how the neutrino event generators work, what can be learned from electron-nucleus interactions and how each underlying physics process - from quasi-elastic to deep inelastic scattering - is understood today. We then emphasize how our understanding must improve to meet the demands of future experiments. With every topic we find that the challenges can be met only with the active support and collaboration among specialists in strong interactions and electroweak physics that include theorists and experimentalists from both the nuclear and high energy physics communities.« less

  18. Noninvasive Online Measurement of Genome Lengths of Mammalian Tissues in Bulk by 14 MeV Neutron Atometry

    NASA Astrophysics Data System (ADS)

    Maglich, Bogdan; Radovic, Anna; Druey, Christian

    2012-10-01

    Genome length, L=, no. of DNA nucleotide base pairs in cell of bovine (b) and porcine (p) tissues, closest to human genome, were hitherto measured by genomic sequencing Lb=3, Lp=2.7 Giga base pairs [1,2] (Gbp) errors not given. - We report measurements of Lb/Lp and Lb, Lp without sequencing by atometry [3,4]. No. of O and C atoms, N, in nucleotide molecules, was obtained from prompt γ rate, G, emitted in inel. scatt. 14 MeV neutrons, with nuclei of C, O, in nucleotide molecule. Since G prop. N, Lb/Lp=Gb/Gp. p and b meat was irradiated for 30'. From msd G we obtained Lb /Lp=1.28±0.02 16% greater than [1,2]. We got absolute Lb=1.65/f, Lp=1.28/f Gbp, 0.3

  19. 41 CFR 50-204.34 - AEC licensees-AEC contractors operating AEC plants and facilities-AEC agreement State licensees...

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... material, or special nuclear material, as defined in the Atomic Energy Act of 1954, as amended, under a license issued by the Atomic Energy Commission and in accordance with the requirements of 10 CFR part 20... contract with the Atomic Energy Commission for the operation of AEC plants and facilities and in accordance...

  20. 41 CFR 50-204.34 - AEC licensees-AEC contractors operating AEC plants and facilities-AEC agreement State licensees...

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... material, or special nuclear material, as defined in the Atomic Energy Act of 1954, as amended, under a license issued by the Atomic Energy Commission and in accordance with the requirements of 10 CFR part 20... contract with the Atomic Energy Commission for the operation of AEC plants and facilities and in accordance...

  1. Data needs for X-ray astronomy satellites

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kallman, T.

    I review the current status of atomic data for X-ray astronomy satellites. This includes some of the astrophysical issues which can be addressed, current modeling and analysis techniques, computational tools, the limitations imposed by currently available atomic data, and the validity of standard assumptions. I also discuss the future: challenges associated with future missions and goals for atomic data collection.

  2. Effects of ionizing radiation on the light sensing elements of the retina. [Structural and physiological effects of carbon, helium, and neon ions on rods and cones of salamanders and mice

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Malachowski, M.J.

    1978-07-01

    This investigation was undertaken to quantitate possible morphological and physiological effects of particles of high linear energy transfer on the retina, in comparison with x-ray effects. The particles used were accelerated atomic nuclei of helium, carbon, and neon at kinetic energies of several hundred MeV/nucleon. For morphological studies, scanning and transmission electron microscopy and light microscopy were used. Physiological studies consisted of autoradiographic data of the rate of incorporation of labeled protein in the structures (opsin) of the outer segment of visual cells. Structural changes were found in the nuclei, as well as the inner and outer segments of visualmore » cells, rods and cones. At a low dose of 10 rad, x rays and helium had no statistically significant morphological effects, but carbon and neon beams did cause significant degeneration of individual cells, pointing to the existence of a linear dose--effect relationship. At high doses of several hundred rads, a Pathologic Index determined the relative biological effectiveness of neon against alpha particles to have a value of greater than 6. The severity of effects per particle increased with atomic number. Labeling studies demonstrated a decreased rate of incorporation of labeled proteins in the structural organization of the outer segments of visual rods. The rate of self-renewal of visual rod discs was punctuated by irradiation and the structures themselves were depleted of amino acids. A model of rod discs (metabolic and catabolic) was postulated for correlated early and late effects to high and low doses.« less

  3. Selective excitation enables assignment of proton resonances and {sup 1}H-{sup 1}H distance measurement in ultrafast magic angle spinning solid state NMR spectroscopy

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Zhang, Rongchun; Ramamoorthy, Ayyalusamy, E-mail: ramamoor@umich.edu

    2015-07-21

    Remarkable developments in ultrafast magic angle spinning (MAS) solid-state NMR spectroscopy enabled proton-based high-resolution multidimensional experiments on solids. To fully utilize the benefits rendered by proton-based ultrafast MAS experiments, assignment of {sup 1}H resonances becomes absolutely necessary. Herein, we propose an approach to identify different proton peaks by using dipolar-coupled heteronuclei such as {sup 13}C or {sup 15}N. In this method, after the initial preparation of proton magnetization and cross-polarization to {sup 13}C nuclei, transverse magnetization of desired {sup 13}C nuclei is selectively prepared by using DANTE (Delays Alternating with Nutations for Tailored Excitation) sequence and then, it is transferredmore » to bonded protons with a short-contact-time cross polarization. Our experimental results demonstrate that protons bonded to specific {sup 13}C atoms can be identified and overlapping proton peaks can also be assigned. In contrast to the regular 2D HETCOR experiment, only a few 1D experiments are required for the complete assignment of peaks in the proton spectrum. Furthermore, the finite-pulse radio frequency driven recoupling sequence could be incorporated right after the selection of specific proton signals to monitor the intensity buildup for other proton signals. This enables the extraction of {sup 1}H-{sup 1}H distances between different pairs of protons. Therefore, we believe that the proposed method will greatly aid in fast assignment of peaks in proton spectra and will be useful in the development of proton-based multi-dimensional solid-state NMR experiments to study atomic-level resolution structure and dynamics of solids.« less

  4. Discrimination Between Cervical Cancer Cells and Normal Cervical Cells Based on Longitudinal Elasticity Using Atomic Force Microscopy

    NASA Astrophysics Data System (ADS)

    Zhao, Xueqin; Zhong, Yunxin; Ye, Ting; Wang, Dajing; Mao, Bingwei

    2015-12-01

    The mechanical properties of cells are considered promising biomarkers for the early diagnosis of cancer. Recently, atomic force microscopy (AFM)-based nanoindentation technology has been utilized for the examination of cell cortex mechanics in order to distinguish malignant cells from normal cells. However, few attempts to evaluate the biomechanical properties of cells have focused on the quantification of the non-homogeneous longitudinal elasticity of cellular structures. In the present study, we applied a variation of the method of Carl and Schillers to investigate the differences between longitudinal elasticity of human cervical squamous carcinoma cells (CaSki) and normal cervical epithelial cells (CRL2614) using AFM. The results reveal a three-layer heterogeneous structure in the probing volume of both cell types studied. CaSki cells exhibited a lower whole-cell stiffness and a softer nuclei zone compared to the normal counterpart cells. Moreover, a better differentiated cytoskeleton was found in the inner cytoplasm/nuclei zone of the normal CRL2614 cells, whereas a deeper cytoskeletal distribution was observed in the probing volume of the cancerous counterparts. The sensitive cortical panel of CaSki cells, with a modulus of 0.35~0.47 kPa, was located at 237~225 nm; in normal cells, the elasticity was 1.20~1.32 kPa at 113~128 nm. The present improved method may be validated using the conventional Hertz-Sneddon method, which is widely reported in the literature. In conclusion, our results enable the quantification of the heterogeneous longitudinal elasticity of cancer cells, in particular the correlation with the corresponding depth. Preliminary results indicate that our method may potentially be applied to improve the detection of cancerous cells and provide insights into the pathophysiology of the disease.

  5. [Study of hydrogen bonds in the "catalytic triad" of trypsin by NMR spectra at 1H, 13C, and 15N nuclei].

    PubMed

    Golubeb, N S; Gindin, V A; Ligaĭ, S S; Smirnov, S N

    1994-05-01

    The 1H and 13C NMR of trypsin stabilized by chemical modification with a hydrophilic polymer have been obtained in a wide range of pH (1.0-11.0). The spectral features referred to some nuclei of the "catalytic triad" have been identified using different NMR techniques as well as chemical modification with selective reagents. It was found that the monoprotonation of this system results in a quasi-symmetrical hydrogen bond formed between the basic groups which provided explanation for the discrepancies between the experimental findings obtained by different authors concerning the protonation site in this catalytic system. Simulation of the catalytic triad by a 15N-labelled low molecular model suggests that an increase in the OH-group acidity is unaccompanied by a discrete double proton transfer; however, a smooth shift of the bridging protons from one basic atom to another occurs with quasi-symmetrical hydrogen bonds formed in intermediate cases. On the basis of experimental data a new concept has been proposed for the mechanism of acid-base catalysis performed by pains of weak basic groups, such as His-Im and Asp(Glu)-COO- (pKa = 3-7) which are not capable of proton abstraction from alcoholic or water OH-groups (pKa > 13). The catalysis may consist in changing the charge densities on the reacting groups due to strong H-bonding and, on the other hand, in facilitating the free movement of a proton in the field of several basic atoms when going along the reaction coordinate. The energy of very strong hydrogen bonds thus formed diminishes the activation energy of the reaction.

  6. Study of photon emission by electron capture during solar nuclei acceleration. 2: Delimitation of conditions for charge transfert establishment

    NASA Technical Reports Server (NTRS)

    Perez-Peraza, J.; Alvarez, M.; Gallegos, A.

    1985-01-01

    The conditions for establishment of charge transfer during acceleration of nuclei up to Fe, for typical conditions of solar flare regions T = 5 x 10 to the 3rd power to 2.5 x 10 to the 8th power degrees K were explored. Results show that such conditions are widely assorted, depending on the acceleration mechanism, the kind of projections and their velocity, the target elements, the source temperature and consequently on the degree of ionization of matter and the local charge state of the accelerated ions. Nevertheless, in spite of that assorted behavior, there are some general tendencies that can be summarized as follows. In atomic H electron capture is systematically established from thermal energies up to high energies, whatever the element and for both acceleration process. For a given element and fixed temperature (T), the probability and energy domain of electron capture and loss with Fermi are higher than with Betatron acceleration. For a given acceleration process the heavier the ion the higher the probability and the wider the energy range for electron capture and loss. For given acceleration mechanism and fixed element the importance and energy domain of capture and loss increase with T: for those reasons, the energy range of charge equilibrium (illustrated with solid lines on the next figs.) is wider with Fermi and increases with temperature and atomic number of projectiles. For the same reasons, electron loss is smaller while the lighter the element, the lower the temperature and the Betatron process, such that there are conditions for which electron loss is not allowed at low energies, but only electron capture is established.

  7. Electron density distribution in BaPb{sub 1-x}Sb{sub x}O{sub 3} superconducting oxides studied by double nuclear magnetic resonance methods

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Piskunov, Yu. V., E-mail: piskunov@imp.uran.ru; Ogloblichev, V. V.; Arapova, I. Yu.

    2011-11-15

    The effect of charge disorder on the formation of an inhomogeneous state of the electron system in the conduction band in BaPb{sub 1-x}Sb{sub x}O{sub 3} superconducting oxides is investigated experimentally by NMR methods. The NMR spectra of {sup 17}O are measured systematically, and the contributions from {sup 17}O atoms with different cation nearest surroundings are identified. It is found that microscopic regions with an elevated spin density of charge carriers are formed within two coordination spheres near antimony ions. Nuclei of the superconducting phase of the oxide (regions with an elevated antimony concentration) microscopically distributed over the sample are detectedmore » in compounds with x = 0.25 and 0.33. Experiments in which a double resonance signal of the spin echo of {sup 17}O-{sup 207}Pb and {sup 17}O-{sup 121}Sb are measured in the metal phase of BaPb{sub 1-x}Sb{sub x}O{sub 3} oxides are carried out for the first time. The constants of indirect heteronuclear spin-spin {sup 17}O-{sup 207}Pb interaction are determined as functions of the local Knight shift {sub 207}Ks. The estimates of the constants of the indirect interaction between the nuclei of the nearest neighbors (O-Pb and Pb-Pb atoms) and analysis of evolution of the NMR spectra of {sup 17}O upon a change in the antimony concentration are convincing evidence in favor of the development of a microscopically inhomogeneous state of the electron system in the metal phase of BaPb{sub 1-x}Sb{sub x}O{sub 3} oxides.« less

  8. Charge radii and electromagnetic moments of At-211195

    NASA Astrophysics Data System (ADS)

    Cubiss, J. G.; Barzakh, A. E.; Seliverstov, M. D.; Andreyev, A. N.; Andel, B.; Antalic, S.; Ascher, P.; Atanasov, D.; Beck, D.; Bieroń, J.; Blaum, K.; Borgmann, Ch.; Breitenfeldt, M.; Capponi, L.; Cocolios, T. E.; Day Goodacre, T.; Derkx, X.; De Witte, H.; Elseviers, J.; Fedorov, D. V.; Fedosseev, V. N.; Fritzsche, S.; Gaffney, L. P.; George, S.; Ghys, L.; Heßberger, F. P.; Huyse, M.; Imai, N.; Kalaninová, Z.; Kisler, D.; Köster, U.; Kowalska, M.; Kreim, S.; Lane, J. F. W.; Liberati, V.; Lunney, D.; Lynch, K. M.; Manea, V.; Marsh, B. A.; Mitsuoka, S.; Molkanov, P. L.; Nagame, Y.; Neidherr, D.; Nishio, K.; Ota, S.; Pauwels, D.; Popescu, L.; Radulov, D.; Rapisarda, E.; Revill, J. P.; Rosenbusch, M.; Rossel, R. E.; Rothe, S.; Sandhu, K.; Schweikhard, L.; Sels, S.; Truesdale, V. L.; Van Beveren, C.; Van den Bergh, P.; Wakabayashi, Y.; Van Duppen, P.; Wendt, K. D. A.; Wienholtz, F.; Whitmore, B. W.; Wilson, G. L.; Wolf, R. N.; Zuber, K.

    2018-05-01

    Hyperfine-structure parameters and isotope shifts of At-211195 have been measured for the first time at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy method. The hyperfine structures of isotopes were recorded using a triad of experimental techniques for monitoring the photo-ion current. The Multi-Reflection Time-of-Flight Mass Spectrometer, in connection with a high-resolution electron multiplier, was used as an ion-counting setup for isotopes that either were affected by strong isobaric contamination or possessed a long half-life; the ISOLDE Faraday cups were used for cases with high-intensity beams; and the Windmill decay station was used for short-lived, predominantly α -decaying nuclei. The electromagnetic moments and changes in the mean-square charge radii of the astatine nuclei have been extracted from the measured hyperfine-structure constants and isotope shifts. This was only made possible by dedicated state-of-the-art large-scale atomic computations of the electronic factors and the specific mass shift of atomic transitions in astatine that are needed for these extractions. By comparison with systematics, it was possible to assess the reliability of the results of these calculations and their ascribed uncertainties. A strong deviation in the ground-state mean-square charge radii of the lightest astatine isotopes, from the trend of the (spherical) lead isotopes, is interpreted as the result of an onset of deformation. This behavior bears a resemblance to the deviation observed in the isotonic polonium isotopes. Cases for shape coexistence have been identified in At,199197, for which a significant difference in the charge radii for ground (9 /2- ) and isomeric (1 /2+ ) states has been observed.

  9. Connections of the Auditory Brainstem in a Songbird, Taeniopygia guttata. II. Projections of Nucleus Angularis and Nucleus Laminaris to the Superior Olive and Lateral Lemniscal Nuclei

    PubMed Central

    Krützfeldt, Nils O.E.; Logerot, Priscilla; Kubke, M. Fabiana; Wild, J. Martin

    2013-01-01

    Three nuclei of the lateral lemniscus are present in the zebra finch, ventral (LLV), intermediate (LLI), and dorsal (LLD). LLV is separate from the superior olive (OS): it lies closer to the spinal lemniscus and extends much further rostrally around the pontine periphery. LLI extends from a caudal position ventrolateral to the principal sensory trigeminal nucleus (LLIc) to a rostral position medial to the ventrolateral parabrachial nucleus (LLIr). LLD consists of posterior (LLDp) and anterior (LLDa) parts, which are largely coextensive rostrocaudally, although LLDa lies medial to LLDp. All nuclei are identifiable on the basis of cytochrome oxidase activity. The cochlear nucleus angularis (NA) and the third-order nucleus laminaris (NL) project on OS predominantly ipsilaterally, on LLV and LLI predominantly contralaterally, and on LLD contralaterally only. The NA projections are heavier than those of NL and differ from them primarily in their terminations within LLD: NA projects to LLDp, whereas NL projects to LLDa. In this the projections are similar to those in the barn owl (Takahashi and Konishi [1988] J Comp Neurol 274:212–238), in which time and intensity pathways remain separate as far as the central nucleus of the inferior colliculus (MLd). In contrast, in the zebra finch, although NA and NL projections remain separate within LLD, the projections of LLDa and LLDp become intermixed within MLd (Wild et al., J Comp Neurol, this issue), consistent with the intermixing of the direct NA and NL projections to MLd (Krützfeldt et al., J Comp Neurol, this issue). J. Comp. Neurol. 518:2135–2148, 2010. PMID:20394062

  10. Mass predictions of atomic nuclei in the infinite nuclear matter model

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Nayak, R.C., E-mail: rcnayak00@yahoo.com; Satpathy, L., E-mail: satpathy@iopb.res.in

    We present here the mass excesses, binding energies, one- and two-neutron, one- and two-proton and {alpha}-particle separation energies of 6727 nuclei in the ranges 4{<=}Z{<=}120 and 8{<=}A{<=}303 calculated in the infinite nuclear matter model. Compared to our predictions of 1999 mass table, the present ones are obtained using larger data base of 2003 mass table of Wapstra and Audi and resorting to higher accuracy in the solutions of the {eta}-differential equations of the INM model. The local energy {eta}'s supposed to carry signature of the characteristic properties of nuclei are found to possess the predictive capability. In fact {eta}-systematics revealmore » new magic numbers in the drip-line regions giving rise to new islands of stability supported by relativistic mean field theoretic calculations. This is a manifestation of a new phenomenon where shell-effect overcomes the instability due to repulsive components of the nucleon-nucleon force broadening the stability peninsula. The two-neutron separation energy-systematics derived from the present mass predictions reveal a general new feature for the existence of islands of inversion in the exotic neutron-rich regions of nuclear landscape, apart from supporting the presently known islands around {sup 31}Na and {sup 62}Ti. The five global parameters representing the properties of infinite nuclear matter, the surface, the Coulomb and the pairing terms are retained as per our 1999 mass table. The root-mean-square deviation of the present mass-fit to 2198 known masses is 342 keV, while the mean deviation is 1.3 keV, reminiscent of no left-over systematic effects. This is a substantive improvement over our 1999 mass table having rms deviation of 401 keV and mean deviation of 9 keV for 1884 data nuclei.« less

  11. An Adaptive QSE-reduced Nuclear Reaction Network for Silicon Burning

    NASA Astrophysics Data System (ADS)

    Parete-Koon, Suzanne; Hix, W.; Thielemann, F.

    2008-03-01

    The nuclei of the "iron peak" are formed in massive stars shortly before core collapse and during their supernova outbursts as well as during thermonuclear supernovae. Complete and incomplete silicon burning during these events are responsible for the production of a wide range of nuclei with atomic mass numbers from 28 to 64. Because of the large number of nuclei involved, accurate modeling of silicon burning is computationally expensive. However, examination of the physics of silicon burning has revealed that the nuclear evolution is dominated by large groups of nuclei in mutual equilibrium. We present an improvement on our hybrid equilibrium-network scheme which takes advantage of this quasi-equilibrium in order to reduce the number of independent variables calculated. Because the size and membership of these groups vary as the temperature, density and electron faction change, achieving maximal efficiency requires dynamic adjustment of group number and membership. Toward this end, we are implementing a scheme beginning with a single QSE (NSE) group at appropriately high temperature, then progressing through 2, 3 and 4 group stages (with successively more independent variables) as temperature declines. This combination allows accurate prediction of the nuclear abundance evolution, deleptonization and energy generation at a further reduced computational cost when compared to a conventional nuclear reaction network or our previous 3 fixed group QSE-reduced network. During silicon burning, the resultant QSE-reduced network is up to 20 times faster than the full network it replaces without significant loss of accuracy. These reductions in computational cost and the number of species evolved make QSE-reduced networks well suited for inclusion within hydrodynamic simulations, particularly in multi-dimensional applications. This work has been supported by the National Science Foundation, by the Department of Energy's Scientic Discovery through Advanced Computing Programs, and by the Joint Institute for Heavy Ion Research at ORNL.

  12. Definition of molecular structure: by choice or by appeal to observation?

    PubMed

    Bader, Richard F W

    2010-07-22

    There are two schools of thought in chemistry: one derived from the valence bond and molecular orbital models of bonding, the other appealing directly to the measurable electron density and the quantum mechanical theorems that determine its behavior, an approach embodied in the quantum theory of atoms in molecules, QTAIM. No one questions the validity of the former approach, and indeed molecular orbital models and QTAIM play complementary roles, the models finding expression in the principles of physics. However, some orbital proponents step beyond the models to impose their personal stamp on their use in interpretive chemistry, by denying the possible existence of a physical basis for the concepts of chemistry. This places them at odds with QTAIM, whose very existence stems from the discovery in the observable topology of the electron density, the definitions of atoms, of the bonding between atoms and hence of molecular structure. Relating these concepts to the electron density provides the necessary link for their ultimate quantum definition. This paper explores in depth the possible causes of the difficulties some have in accepting the quantum basis of structure beginning with the arguments associated with the acceptance of a "bond path" as a criterion for bonding. This identification is based on the finding that all classical structures may be mapped onto molecular graphs consisting of bond paths linking neighboring atoms, a mapping that has no known exceptions and one that is further bolstered by the finding that there are no examples of "missing bond paths". Difficulties arise when the quantum concept is applied to systems that are not amenable to the classical models of bonding. Thus one is faced with the recurring dilemma of science, of having to escape the constraints of a model that requires a change in the existing paradigm, a process that has been in operation since the discovery of new and novel structures necessitated the extension of the Lewis model and the octet rule. The paper reviews all facets of bonding beginning with the work of Pauling and Slater in their accounting for crystal structures, taking note of Pauling's advocating possible bonding between large anions. Many examples of nonbonded or van der Waals interactions are considered from both points of view. The final section deals with the consequences of the realization that bonded quantum atoms that share an interatomic surface do not "overlap". The time has come for entering students of chemistry to be taught that the electron density can be seen, touched, and measured and that the chemical structures they learn are in fact the tracings of "bonds" onto lines of maximum density that link bonded nuclei. Matter, as we perceive it, is bound by the electrostatic force of attraction between the nuclei and the electron density.

  13. Chapter 6 Quantum Mechanical Methods for Loss-Excitation and Loss-Ionization in Fast Ion-Atom Collisions

    NASA Astrophysics Data System (ADS)

    Belkic, Dzevad

    Inelastic collisions between bare nuclei and hydrogen-like atomic systems are characterized by three main channels: electron capture, excitation, and ionization. Capture dominates at lower energies, whereas excitation and ionization prevail at higher impact energies. At intermediate energies and in the region of resonant scattering near the Massey peak, all three channels become competitive. For dressed or clothed nuclei possessing electrons, such as hydrogen-like ions, several additional channels open up, including electron loss (projectile ionization or stripping). The most important aspect of electron loss is the competition between one- and two-electron processes. Here, in a typical one-electron process, the projectile emits an electron, whereas the target final and initial states are the same. A prototype of double-electron transitions in loss processes is projectile ionization accompanied with an alteration of the target state. In such a two-electron process, the target could be excited or ionized. The relative importance of these loss channels with single- and double-electron transitions involving collisions of dressed projectiles with atomic systems is also strongly dependent on the value of the impact energy. Moreover, impact energies determine which theoretical method is likely to be more appropriate to use for predictions of cross sections. At low energies, an expansion of total scattering wave functions in terms of molecular orbitals is adequate. This is because the projectile spends considerable time in the vicinity of the target, and as a result, a compound system comprised of the projectile and the target can be formed in a metastable molecular state which is prone to decay. At high energies, a perturbation series expansion is more appropriate in terms of powers of interaction potentials. In the intermediate energy region, atomic orbitals are often used with success while expanding the total scattering wave functions. The present work is focused on quantum mechanical perturbation theories applied to electron loss collisions involving two hydrogen-like atoms. Both the one- and two-electron transitions (target unaffected by collision, as well as loss-ionization) are thoroughly examined in various intervals of impact energies varying from the threshold via the Massey peak to the Bethe asymptotic region. Systematics are established for the fast, simple, and accurate computations of cross sections for loss-excitation and loss-ionization accounting for the entire spectra of all four particles, including two free electrons and two free protons. The expounded algorithmic strategy of quantum mechanical methodologies is of great importance for wide applications to particle transport physics, especially in fusion research and hadron radiotherapy. This should advantageously replace the current overwhelming tendency in these fields for using phenomenological modeling with artificial functions extracted from fitting the existing experimental/theoretical data bases for cross sections.

  14. Connections of the Auditory Brainstem in a Songbird, Taeniopygia guttata. III. Projections of the Superior Olive and Lateral Lemniscal Nuclei

    PubMed Central

    Wild, J. Martin; Krützfeldt, Nils O.E.; Kubke, M. Fabiana

    2013-01-01

    Sequential to companion articles that report the projections of the cochlear nucleus angularis (NA) and the third-order nucleus laminaris (NL) to the central nucleus of the inferior colliculus (MLd) and to the superior olive (OS) and lateral lemniscal nuclei (LLV, LLI, and LLD) (Krützfeldt et al., J Comp Neurol, this issue), we here describe the projections of the latter group of nuclei using standard tract-tracing methods. OS projects on LLV and both have further ascending projections on LLI, LLD, and MLd. LLV also provides auditory input to the song system, via nucleus uvaeformis, and to the thalamo-telencephalic auditory system, via nucleus ovoidalis (Ov), thus bypassing MLd. The two divisions of LLD (LLDa and LLDp) project across the midline via the commissure of Probst each to innervate the homologous contralateral nucleus and MLd. Both, particularly LLDp, also project on Ov. Injections in LLD and LLV resulted in anterograde labeling of caudal nucleus basorostralis (Bas) in the frontal telencephalon, but retrograde tracing so far suggests that only LLI is a real source of this projection (Wild and Farabaugh [1996] J Comp Neurol 365:306–328). OS and LLV also have descending projections on the ipsilateral NA, NM, and NL, and LLV also projects on OS. The ascending inputs to MLd and more rostral nuclei may contribute importantly to mechanisms of auditory pattern (song) recognition. Consistent with previous studies, some of the descending projections may be inhibitory. PMID:20394063

  15. Two-phase deep convolutional neural network for reducing class skewness in histopathological images based breast cancer detection.

    PubMed

    Wahab, Noorul; Khan, Asifullah; Lee, Yeon Soo

    2017-06-01

    Different types of breast cancer are affecting lives of women across the world. Common types include Ductal carcinoma in situ (DCIS), Invasive ductal carcinoma (IDC), Tubular carcinoma, Medullary carcinoma, and Invasive lobular carcinoma (ILC). While detecting cancer, one important factor is mitotic count - showing how rapidly the cells are dividing. But the class imbalance problem, due to the small number of mitotic nuclei in comparison to the overwhelming number of non-mitotic nuclei, affects the performance of classification models. This work presents a two-phase model to mitigate the class biasness issue while classifying mitotic and non-mitotic nuclei in breast cancer histopathology images through a deep convolutional neural network (CNN). First, nuclei are segmented out using blue ratio and global binary thresholding. In Phase-1 a CNN is then trained on the segmented out 80×80 pixel patches based on a standard dataset. Hard non-mitotic examples are identified and augmented; mitotic examples are oversampled by rotation and flipping; whereas non-mitotic examples are undersampled by blue ratio histogram based k-means clustering. Based on this information from Phase-1, the dataset is modified for Phase-2 in order to reduce the effects of class imbalance. The proposed CNN architecture and data balancing technique yielded an F-measure of 0.79, and outperformed all the methods relying on specific handcrafted features, as well as those using a combination of handcrafted and CNN-generated features. Copyright © 2017 Elsevier Ltd. All rights reserved.

  16. Cosmology beyond the Standard Model

    NASA Astrophysics Data System (ADS)

    Wells, Christopher M.

    The Standard Model of Cosmology, like its particle physics counterpart, is incomplete in its present form theoretically and observationally. Additional structure, in the form of an early period of accelerated expansion (inflation), is suggested by the special initial conditions required to produce the visible universe. Furthermore, a wide variety of indirect observations indicate that 80% of the mass in the universe is dark. In this thesis, we construct a class of inflation models free from the usual pathologies. In particular, we build a novel realization of hybrid inflation, in which both the inflaton and waterfall degrees of freedom are moduli of a higher dimensional compactification. Because the inflationary fields are realized as global degrees of freedom in the extra dimension, they are protected from the 4D quantum corrections that would otherwise spoil inflation. Via the Ads/CFT correspondence we can relate our construction to a dual theory of composite inflationary degrees of freedom. We then turn to studying the problem of missing matter in the Standard Cosmology. Despite an abundance of indirect observations of dark matter, direct detection experiments have produced conflicting results which seem to point to a more complicated dark sector. In this thesis, we propose that dark matter be made up primarily of non-relativistic bound states, i.e. dark atoms. We explore the atomic parameter space allowed by the demands that dark matter is predominantly atomic and that the dark atoms and ions satisfy observational bounds on dark matter self-interactions. We then study possible interactions between dark matter and normal matter such that dark atoms scatter inelastically from nuclei in direct detection experiments.

  17. Beating Homogeneous Nucleation and Tuning Atomic Ordering in Glass-Forming Metals by Nanocalorimetry.

    PubMed

    Zhao, Bingge; Yang, Bin; Abyzov, Alexander S; Schmelzer, Jürn W P; Rodríguez-Viejo, Javier; Zhai, Qijie; Schick, Christoph; Gao, Yulai

    2017-12-13

    In this paper, the amorphous Ce 68 Al 10 Cu 20 Co 2 (atom %) alloy was in situ prepared by nanocalorimetry. The high cooling and heating rates accessible with this technique facilitate the suppression of crystallization on cooling and the identification of homogeneous nucleation. Different from the generally accepted notion that metallic glasses form just by avoiding crystallization, the role of nucleation and growth in the crystallization behavior of amorphous alloys is specified, allowing an access to the ideal metallic glass free of nuclei. Local atomic configurations are fundamentally significant to unravel the glass forming ability (GFA) and phase transitions in metallic glasses. For this reason, isothermal annealing near T g from 0.001 s to 25,000 s following quenching becomes the strategy to tune local atomic configurations and facilitate an amorphous alloy, a mixed glassy-nanocrystalline state, and a crystalline sample successively. On the basis of the evolution of crystallization enthalpy and overall latent heat on reheating, we quantify the underlying mechanism for the isothermal nucleation and crystallization of amorphous alloys. With Johnson-Mehl-Avrami method, it is demonstrated that the coexistence of homogeneous and heterogeneous nucleation contributes to the isothermal crystallization of glass. Heterogeneous rather than homogeneous nucleation dominates the isothermal crystallization of the undercooled liquid. For the mixed glassy-nanocrystalline structure, an extraordinary kinetic stability of the residual glass is validated, which is ascribed to the denser packed interface between amorphous phase and ordered nanocrystals. Tailoring the amorphous structure by nanocalorimetry permits new insights into unraveling GFA and the mechanism that correlates local atomic configurations and phase transitions in metallic glasses.

  18. Nanoscale Nucleation and Growth of Electrodeposited Lithium Metal

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Pei, Allen; Zheng, Guangyuan; Shi, Feifei

    Lithium metal has re-emerged as an exciting anode for high energy lithium-ion batteries due to its high specific capacity of 3860 mAh g -1 and lowest electrochemical potential of all known materials. However, lithium has been plagued by the issues of dendrite formation, high chemical reactivity with electrolyte, and infinite relative volume expansion during plating and stripping, which present safety hazards and low cycling efficiency in batteries with lithium metal electrodes. There have been a lot of recent studies on Li metal although little work has focused on the initial nucleation and growth behavior of Li metal, neglecting a criticalmore » fundamental scientific foundation of Li plating. Here, we study experimentally the morphology of lithium in the early stages of nucleation and growth on planar copper electrodes in liquid organic electrolyte. We elucidate the dependence of lithium nuclei size, shape, and areal density on current rate, consistent with classical nucleation and growth theory. We found that the nuclei size is proportional to the inverse of overpotential and the number density of nuclei is proportional to the cubic power of overpotential. Finally, based on this understanding, we propose a strategy to increase the uniformity of electrodeposited lithium on the electrode surface.« less

  19. Nanoscale Nucleation and Growth of Electrodeposited Lithium Metal

    DOE PAGES

    Pei, Allen; Zheng, Guangyuan; Shi, Feifei; ...

    2017-01-10

    Lithium metal has re-emerged as an exciting anode for high energy lithium-ion batteries due to its high specific capacity of 3860 mAh g -1 and lowest electrochemical potential of all known materials. However, lithium has been plagued by the issues of dendrite formation, high chemical reactivity with electrolyte, and infinite relative volume expansion during plating and stripping, which present safety hazards and low cycling efficiency in batteries with lithium metal electrodes. There have been a lot of recent studies on Li metal although little work has focused on the initial nucleation and growth behavior of Li metal, neglecting a criticalmore » fundamental scientific foundation of Li plating. Here, we study experimentally the morphology of lithium in the early stages of nucleation and growth on planar copper electrodes in liquid organic electrolyte. We elucidate the dependence of lithium nuclei size, shape, and areal density on current rate, consistent with classical nucleation and growth theory. We found that the nuclei size is proportional to the inverse of overpotential and the number density of nuclei is proportional to the cubic power of overpotential. Finally, based on this understanding, we propose a strategy to increase the uniformity of electrodeposited lithium on the electrode surface.« less

  20. Nanoscale Nucleation and Growth of Electrodeposited Lithium Metal.

    PubMed

    Pei, Allen; Zheng, Guangyuan; Shi, Feifei; Li, Yuzhang; Cui, Yi

    2017-02-08

    Lithium metal has re-emerged as an exciting anode for high energy lithium-ion batteries due to its high specific capacity of 3860 mAh g -1 and lowest electrochemical potential of all known materials. However, lithium has been plagued by the issues of dendrite formation, high chemical reactivity with electrolyte, and infinite relative volume expansion during plating and stripping, which present safety hazards and low cycling efficiency in batteries with lithium metal electrodes. There have been a lot of recent studies on Li metal although little work has focused on the initial nucleation and growth behavior of Li metal, neglecting a critical fundamental scientific foundation of Li plating. Here, we study experimentally the morphology of lithium in the early stages of nucleation and growth on planar copper electrodes in liquid organic electrolyte. We elucidate the dependence of lithium nuclei size, shape, and areal density on current rate, consistent with classical nucleation and growth theory. We found that the nuclei size is proportional to the inverse of overpotential and the number density of nuclei is proportional to the cubic power of overpotential. Based on this understanding, we propose a strategy to increase the uniformity of electrodeposited lithium on the electrode surface.

  1. On-the-Fly Generation of Differential Resonance Scattering Probability Distribution Functions for Monte Carlo Codes

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Davidson, Eva E.; Martin, William R.

    Current Monte Carlo codes use one of three models: (1) the asymptotic scattering model, (2) the free gas scattering model, or (3) the S(α,β) model, depending on the neutron energy and the specific Monte Carlo code. This thesis addresses the consequences of using the free gas scattering model, which assumes that the neutron interacts with atoms in thermal motion in a monatomic gas in thermal equilibrium at material temperature, T. Most importantly, the free gas model assumes the scattering cross section is constant over the neutron energy range, which is usually a good approximation for light nuclei, but not formore » heavy nuclei where the scattering cross section may have several resonances in the epithermal region. Several researchers in the field have shown that the exact resonance scattering model is temperaturedependent, and neglecting the resonances in the lower epithermal range can under-predict resonance absorption due to the upscattering phenomenon mentioned above, leading to an over-prediction of keff by several hundred pcm. Existing methods to address this issue involve changing the neutron weights or implementing an extra rejection scheme in the free gas sampling scheme, and these all involve performing the collision analysis in the center-of-mass frame, followed by a conversion back to the laboratory frame to continue the random walk of the neutron. The goal of this paper was to develop a sampling methodology that (1) accounted for the energydependent scattering cross sections in the collision analysis and (2) was performed in the laboratory frame,avoiding the conversion to the center-of-mass frame. The energy dependence of the scattering cross section was modeled with even-ordered polynomials (2nd and 4th order) to approximate the scattering cross section in Blackshaw’s equations for the moments of the differential scattering PDFs. These moments were used to sample the outgoing neutron speed and angle in the laboratory frame on-the-fly during the random walk of the neutron. Results for criticality studies on fuel pin and fuel assembly calculations using methods developed in this dissertation showed very close comparison to results using the reference Dopplerbroadened rejection correction (DBRC) scheme.« less

  2. On-the-Fly Generation of Differential Resonance Scattering Probability Distribution Functions for Monte Carlo Codes

    DOE PAGES

    Davidson, Eva E.; Martin, William R.

    2017-05-26

    Current Monte Carlo codes use one of three models: (1) the asymptotic scattering model, (2) the free gas scattering model, or (3) the S(α,β) model, depending on the neutron energy and the specific Monte Carlo code. This thesis addresses the consequences of using the free gas scattering model, which assumes that the neutron interacts with atoms in thermal motion in a monatomic gas in thermal equilibrium at material temperature, T. Most importantly, the free gas model assumes the scattering cross section is constant over the neutron energy range, which is usually a good approximation for light nuclei, but not formore » heavy nuclei where the scattering cross section may have several resonances in the epithermal region. Several researchers in the field have shown that the exact resonance scattering model is temperaturedependent, and neglecting the resonances in the lower epithermal range can under-predict resonance absorption due to the upscattering phenomenon mentioned above, leading to an over-prediction of keff by several hundred pcm. Existing methods to address this issue involve changing the neutron weights or implementing an extra rejection scheme in the free gas sampling scheme, and these all involve performing the collision analysis in the center-of-mass frame, followed by a conversion back to the laboratory frame to continue the random walk of the neutron. The goal of this paper was to develop a sampling methodology that (1) accounted for the energydependent scattering cross sections in the collision analysis and (2) was performed in the laboratory frame,avoiding the conversion to the center-of-mass frame. The energy dependence of the scattering cross section was modeled with even-ordered polynomials (2nd and 4th order) to approximate the scattering cross section in Blackshaw’s equations for the moments of the differential scattering PDFs. These moments were used to sample the outgoing neutron speed and angle in the laboratory frame on-the-fly during the random walk of the neutron. Results for criticality studies on fuel pin and fuel assembly calculations using methods developed in this dissertation showed very close comparison to results using the reference Dopplerbroadened rejection correction (DBRC) scheme.« less

  3. On the search for the electric dipole moment of strange and charm baryons at LHC

    NASA Astrophysics Data System (ADS)

    Botella, F. J.; Garcia Martin, L. M.; Marangotto, D.; Martinez Vidal, F.; Merli, A.; Neri, N.; Oyanguren, A.; Ruiz Vidal, J.

    2017-03-01

    Permanent electric dipole moments (EDMs) of fundamental particles provide powerful probes for physics beyond the Standard Model. We propose to search for the EDM of strange and charm baryons at LHC, extending the ongoing experimental program on the neutron, muon, atoms, molecules and light nuclei. The EDM of strange Λ baryons, selected from weak decays of charm baryons produced in p p collisions at LHC, can be determined by studying the spin precession in the magnetic field of the detector tracking system. A test of CPT symmetry can be performed by measuring the magnetic dipole moment of Λ and \\overline{Λ} baryons. For short-lived {Λ} ^+c and {Ξ} ^+c baryons, to be produced in a fixed-target experiment using the 7 TeV LHC beam and channeled in a bent crystal, the spin precession is induced by the intense electromagnetic field between crystal atomic planes. The experimental layout based on the LHCb detector and the expected sensitivities in the coming years are discussed.

  4. Ultrafast electron diffraction and electron microscopy: present status and future prospects

    NASA Astrophysics Data System (ADS)

    Ishchenko, A. A.; Aseyev, S. A.; Bagratashvili, V. N.; Panchenko, V. Ya; Ryabov, E. A.

    2014-07-01

    Acting as complementary research tools, high time-resolved spectroscopy and diffractometry techniques proceeding from various physical principles open up new possibilities for studying matter with necessary integration of the 'structure-dynamics-function' triad in physics, chemistry, biology and materials science. Since the 1980s, a new field of research has started at the leading research laboratories, aimed at developing means of filming the coherent dynamics of nuclei in molecules and fast processes in biological objects ('atomic and molecular movies'). The utilization of ultrashort laser pulse sources has significantly modified traditional electron beam approaches to and provided high space-time resolution for the study of materials. Diffraction methods using frame-by-frame filming and the development of the main principles of the study of coherent dynamics of atoms have paved the way to observing wave packet dynamics, the intermediate states of reaction centers, and the dynamics of electrons in molecules, thus allowing a transition from the kinetics to the dynamics of the phase trajectories of molecules in the investigation of chemical reactions.

  5. Demonstration of a Sensitive Method to Measure Nuclear-Spin-Dependent Parity Violation

    NASA Astrophysics Data System (ADS)

    Altuntaş, Emine; Ammon, Jeffrey; Cahn, Sidney B.; DeMille, David

    2018-04-01

    Nuclear-spin-dependent parity violation (NSD-PV) effects in atoms and molecules arise from Z0 boson exchange between electrons and the nucleus, and from the magnetic interaction between electrons and the parity-violating nuclear anapole moment. We demonstrate measurements of NSD-PV that use an enhancement of the effect in diatomic molecules, here using the test system 138Ba 19. Our sensitivity surpasses that of any previous atomic parity violation measurement. We show that systematic errors can be suppressed to at least the level of the present statistical sensitivity. We measure the matrix element W of the NSD-PV interaction with total uncertainty δ W /(2 π )<0.7 Hz , for each of two configurations where W must have different signs. This sensitivity would be sufficient to measure NSD-PV effects of the size anticipated across a wide range of nuclei including 137Ba in 137BaF, where |W |/(2 π )≈5 Hz is expected.

  6. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Garcia Ruiz, R. F.; Bissell, M. L.; Blaum, K.

    Here, despite being a complex many-body system, the atomic nucleus exhibits simple structures for certain ‘magic’ numbers of protons and neutrons. The calcium chain in particular is both unique and puzzling: evidence of doubly magic features are known in 40,48Ca, and recently suggested in two radioactive isotopes, 52,54Ca. Although many properties of experimentally known calcium isotopes have been successfully described by nuclear theory, it is still a challenge to predict the evolution of their charge radii. Here we present the first measurements of the charge radii of 49,51,52Ca, obtained from laser spectroscopy experiments at ISOLDE, CERN. The experimental results aremore » complemented by state-of-the-art theoretical calculations. The large and unexpected increase of the size of the neutron-rich calcium isotopes beyond N = 28 challenges the doubly magic nature of 52Ca and opens new intriguing questions on the evolution of nuclear sizes away from stability, which are of importance for our understanding of neutron-rich atomic nuclei.« less

  7. Meteor research program

    NASA Technical Reports Server (NTRS)

    Southworth, R. B.; Mccrosky, R. E.

    1970-01-01

    An overview of research on radio and radar meteors accomplished during the past decade is presented, and the work of the past year is highlighted. Velocity distribution and mass flux data are obtained for meteors in the range 10 to 0.0001 g, the size believed to be the principal hazard to space missions. The physical characteristics of mass, structure and density, luminosity, and ablation are briefly described, and the formulation of a theory for interactions of ionization and excitation during collision of atomic particles is mentioned. Five classes of meteoroids are identified, including the two of iron and stone meteorites. Stream meteors associated with known comets are Classes A or C, and parent comets of Class B streams are not observed. Class A meteoroids are identified with the core of a cometary nucleus, Class C with less dense surface of the nucleus after sublimation of ices, and Class B with less dense cores of smaller cometary nuclei. Atmospheric meteor phenomena associated with winds and gravity waves, density and temperature, atomic oxygen, and meteor rate changes are mentioned.

  8. Boron Neutron Capture Therapy - A Literature Review

    PubMed Central

    Nedunchezhian, Kavitaa; Thiruppathy, Manigandan; Thirugnanamurthy, Sarumathi

    2016-01-01

    Boron Neutron Capture Therapy (BNCT) is a radiation science which is emerging as a hopeful tool in treating cancer, by selectively concentrating boron compounds in tumour cells and then subjecting the tumour cells to epithermal neutron beam radiation. BNCT bestows upon the nuclear reaction that occurs when Boron-10, a stable isotope, is irradiated with low-energy thermal neutrons to yield α particles (Helium-4) and recoiling lithium-7 nuclei. A large number of 10 Boron (10B) atoms have to be localized on or within neoplastic cells for BNCT to be effective, and an adequate number of thermal neutrons have to be absorbed by the 10B atoms to maintain a lethal 10B (n, α) lithium-7 reaction. The most exclusive property of BNCT is that it can deposit an immense dose gradient between the tumour cells and normal cells. BNCT integrates the fundamental focusing perception of chemotherapy and the gross anatomical localization proposition of traditional radiotherapy. PMID:28209015

  9. Nuclear magnetic and nuclear quadrupole resonance parameters of β-carboline derivatives calculated using density functional theory

    NASA Astrophysics Data System (ADS)

    Ahmadinejad, Neda; Tari, Mostafa Talebi

    2017-04-01

    A density functional theory (DFT) calculations using B3LYP/6-311++G( d,p) method were carried out to investigate the relative stability of the molecules of β-carboline derivatives such as harmaline, harmine, harmalol, harmane and norharmane. Calculated nuclear quadrupole resonance (NQR) parameters were used to determine the 14N nuclear quadrupole coupling constant χ, asymmetry parameter η and EFG tensor ( q zz ). For better understanding of the electronic structure of β-carboline derivatives, natural bond orbital (NBO) analysis, isotropic and anisotropic NMR chemical shieldings were calculated for 14N nuclei using GIAO method for the optimized structures. The NBO analysis shows that pyrrole ring nitrogen (N9) atom has greater tendency than pyridine ring nitrogen (N2) atom to participate in resonance interactions and aromaticity development in the all of these structures. The NMR and NQR parameters were studied in order to find the correlations between electronic structure and the structural stability of the studied molecules.

  10. Communication: Nuclear quadrupole moment-induced Cotton-Mouton effect in noble gas atoms

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Fu, Li-juan; Vaara, Juha, E-mail: juha.vaara@iki.fi; Rizzo, Antonio

    New, high-sensitivity and high-resolution spectroscopic and imaging methods may be developed by exploiting nuclear magneto-optic effects. A first-principles electronic structure formulation of nuclear electric quadrupole moment-induced Cotton-Mouton effect (NQCME) is presented for closed-shell atoms. In NQCME, aligned quadrupole moments alter the index of refraction of the medium along with and perpendicular to the direction of nuclear alignment. The roles of basis-set convergence, electron correlation, and relativistic effects are investigated for three quadrupolar noble gas isotopes: {sup 21}Ne, {sup 83}Kr, and {sup 131}Xe. The magnitude of the resulting ellipticities is predicted to be 10{sup −4}–10{sup −6} rad/(M cm) for fully spin-polarized nuclei.more » These should be detectable in the Voigt setup. Particularly interesting is the case of {sup 131}Xe, in which a high degree of spin polarization can be achieved via spin-exchange optical hyperpolarization.« less

  11. Magnetic interactions at Ce impurities in REMn2Ge2 (RE = La, Ce, Pr, Nd) compounds

    NASA Astrophysics Data System (ADS)

    Bosch-Santos, B.; Cabrera-Pasca, G. A.; Saxena, R. N.; Burimova, A. N.; Carbonari, A. W.

    2018-05-01

    In the work reported in this paper, the temperature dependence of the magnetic hyperfine field (Bh f) at 140Ce nuclei replacing Pr atoms in PrMn2Ge2 compound was measured by the perturbed angular correlation technique to complete the sequence of measurements in REMn2Ge2 (RE = La, Ce, Pr, Nd). Results show an anomalous behavior different from the expected Brillouin curve. A model was used to fit the data showing that the Ce impurity contribution (Bhfimp) to Bhf is negative for NdMn2Ge2 below 210 K. The impurity contribution (Bhfimp) at 0 K for all compounds is much smaller than that for the free Ce3+, showing that the 4f band of Ce is more likely highly hybridized with 5d band of the host. Results show that direction of the localized magnetic moment at Mn atoms strongly affects the exchange interaction at Ce impurities.

  12. Nuclear spectroscopy with Geant4. The superheavy challenge

    NASA Astrophysics Data System (ADS)

    Sarmiento, Luis G.

    2016-12-01

    The simulation toolkit Geant4 was originally developed at CERN for high-energy physics. Over the years it has been established as a swiss army knife not only in particle physics but it has seen an accelerated expansion towards nuclear physics and more recently to medical imaging and γ- and ion- therapy to mention but a handful of new applications. The validity of Geant4 is vast and large across many particles, ions, materials, and physical processes with typically various different models to choose from. Unfortunately, atomic nuclei with atomic number Z > 100 are not properly supported. This is likely due to the rather novelty of the field, its comparably small user base, and scarce evaluated experimental data. To circumvent this situation different workarounds have been used over the years. In this work the simulation toolkit Geant4 will be introduced with its different components and the effort to bring the software to the heavy and superheavy region will be described.

  13. Investigation of the Possibility of Using Nuclear Magnetic Spin Alignment

    NASA Technical Reports Server (NTRS)

    Dent, William V., Jr.

    1998-01-01

    The goal of the program to investigate a "Gasdynamic fusion propulsion system for space exploration" is to develop a fusion propulsion system for a manned mission to the planet mars. A study using Deuterium and Tritium atoms are currently in progress. When these atoms under-go fusion, the resulting neutrons and alpha particles are emitted in random directions (isotropically). The probable direction of emission is equal for all directions, thus resulting in wasted energy, massive shielding and cooling requirements, and serious problems with the physics of achieving fusion. If the nuclear magnetic spin moments of the deuterium and tritium nuclei could be precisely aligned at the moment of fusion, the stream of emitted neutrons could be directed out the rear of the spacecraft for thrust and the alpha particles directed forward into an electromagnet ot produce electricity to continue operating the fusion engine. The following supporting topics are discussed: nuclear magnetic moments and spin precession in magnetic field, nuclear spin quantum mechanics, kinematics of nuclear reactions, and angular distribution of particles.

  14. Nuclear quantum effects of light and heavy water studied by all-electron first principles path integral simulations

    NASA Astrophysics Data System (ADS)

    Machida, Masahiko; Kato, Koichiro; Shiga, Motoyuki

    2018-03-01

    The isotopologs of liquid water, H2O, D2O, and T2O, are studied systematically by first principles PIMD simulations, in which the whole entity of the electrons and nuclei are treated quantum mechanically. The simulation results are in reasonable agreement with available experimental data on isotope effects, in particular, on the peak shift in the radial distributions of H2O and D2O and the shift in the evaporation energies. It is found that, due to differences in nuclear quantum effects, the H atoms in the OH bonds more easily access the dissociative region up to the hydrogen bond center than the D (T) atoms in the OD (OT) bonds. The accuracy and limitation in the use of the current density-functional-theory-based first principles PIMD simulations are also discussed. It is argued that the inclusion of the dispersion correction or relevant improvements in the density functionals are required for the quantitative estimation of isotope effects.

  15. Footprints of electron correlation in strong-field double ionization of Kr close to the sequential-ionization regime

    NASA Astrophysics Data System (ADS)

    Li, Xiaokai; Wang, Chuncheng; Yuan, Zongqiang; Ye, Difa; Ma, Pan; Hu, Wenhui; Luo, Sizuo; Fu, Libin; Ding, Dajun

    2017-09-01

    By combining kinematically complete measurements and a semiclassical Monte Carlo simulation we study the correlated-electron dynamics in the strong-field double ionization of Kr. Interestingly, we find that, as we step into the sequential-ionization regime, there are still signatures of correlation in the two-electron joint momentum spectrum and, more intriguingly, the scaling law of the high-energy tail is completely different from early predictions on the low-Z atom (He). These experimental observations are well reproduced by our generalized semiclassical model adapting a Green-Sellin-Zachor potential. It is revealed that the competition between the screening effect of inner-shell electrons and the Coulomb focusing of nuclei leads to a non-inverse-square central force, which twists the returned electron trajectory at the vicinity of the parent core and thus significantly increases the probability of hard recollisions between two electrons. Our results might have promising applications ranging from accurately retrieving atomic structures to simulating celestial phenomena in the laboratory.

  16. Editorial

    NASA Astrophysics Data System (ADS)

    Rudolph, Dirk; Elding, Lars-Ivar; Fahlander, Claes; Åberg, Sven

    2016-12-01

    Science often develops most vigorously through challenging studies of extreme phenomena. Superheavy elements fall into such a category. What is the heaviest element that can exist in Nature? Driven by the continued search for an anticipated "island of stability" of superheavy atomic nuclei and the understanding of their underlying nuclear (in)stability and atomic structure hence chemical properties, the past decades have seen a tremendous progress in experimental ingenuity and theoretical methodology to study and characterize superheavy elements. Therefore, we are very grateful that the Nobel Foundation [1] approved and, jointly with the Knut and Alice Wallenberg Foundation [2], provided the financial resources to organize and conduct the Nobel Symposium NS160, entitled Chemistry and Physics of Heavy and Superheavy Elements. These symposia "are devoted to areas of science where breakthroughs are occurring or deal with other topics of primary cultural or social significance" [1]. About three symposia are held each year, roughly every fourth symposium promotes a topic in physics as primary research area, and from about every third symposium a contemporary Nobel Price is being awarded.

  17. Nuclear physics for materials technology

    NASA Astrophysics Data System (ADS)

    Conlon, T. W.

    1987-04-01

    Although particle accelerators have traditionally been used to further our knowledge of nuclear physics, the last decade or so has seen a rapid growth of their involvement in materials technology — both to modify materials and to provide analytical information at the atomic level that cannot be obtained in other ways. The deployment of ion beams in these areas has occurred in three phases: first the exploitation of keV ion beams (in ion implantation and SIMS) then MeV light ion beams (using RBS, NRA, PIXE analysis and TLA) and currently MeV heavy ion beams, together with the associated fast recoil atoms and nuclei that they produce in interactions with materials. This trend has been accompanied by the gradual assimilation of methods such as energy analysis, microbeam focussing, particle identification, time of flight and coincidence techniques, etc., which were first developed for experimental nuclear physics use. Current examples of developments in the MeV range relevant to phases 2 and 3 are given.

  18. Basic Equations Interrelate Atomic and Nuclear Properties to Patterns at the Size Scales of the Cosmos, Extended Clusters of Galaxies, Galaxies, and Nebulae

    NASA Astrophysics Data System (ADS)

    Allen, Rob

    2016-09-01

    Structures within molecules and nuclei have relationships to astronomical patterns. The COBE cosmic scale plots, and large scale surveys of galaxy clusters have patterns also repeating and well known at atomic scales. The Induction, Strong Force, and Nuclear Binding Energy Periods within the Big Bang are revealed to have played roles in the formation of these large scale distributions. Equations related to the enormous patterns also model chemical bonds and likely nucleus and nucleon substructures. ratios of the forces that include gravity are accurately calculated from the distributions and shapes. In addition, particle masses and a great many physical constants can be derived with precision and accuracy from astrophysical shapes. A few very basic numbers can do modelling from nucleon internals to molecules to super novae, and up to the Visible Universe. Equations are also provided along with possible structural configurations for some Cold Dark Matter and Dark Energy.

  19. Unexpectedly large charge radii of neutron-rich calcium isotopes

    DOE PAGES

    Garcia Ruiz, R. F.; Bissell, M. L.; Blaum, K.; ...

    2016-02-08

    Here, despite being a complex many-body system, the atomic nucleus exhibits simple structures for certain ‘magic’ numbers of protons and neutrons. The calcium chain in particular is both unique and puzzling: evidence of doubly magic features are known in 40,48Ca, and recently suggested in two radioactive isotopes, 52,54Ca. Although many properties of experimentally known calcium isotopes have been successfully described by nuclear theory, it is still a challenge to predict the evolution of their charge radii. Here we present the first measurements of the charge radii of 49,51,52Ca, obtained from laser spectroscopy experiments at ISOLDE, CERN. The experimental results aremore » complemented by state-of-the-art theoretical calculations. The large and unexpected increase of the size of the neutron-rich calcium isotopes beyond N = 28 challenges the doubly magic nature of 52Ca and opens new intriguing questions on the evolution of nuclear sizes away from stability, which are of importance for our understanding of neutron-rich atomic nuclei.« less

  20. Nucleosynthesis: Stellar and Solar Abundances and Atomic Data

    NASA Technical Reports Server (NTRS)

    Cowan, John J.; Lawler, James E.; Sneden, Christopher; DenHartog, E. A.; Collier, Jason; Dodge, Homer L.

    2006-01-01

    Abundance observations indicate the presence of often surprisingly large amounts of neutron capture (i.e., s- and r-process) elements in old Galactic halo and globular cluster stars. These observations provide insight into the nature of the earliest generations of stars in the Galaxy the progenitors of the halo stars responsible for neutron-capture synthesis. Comparisons of abundance trends can be used to understand the chemical evolution of the Galaxy and the nature of heavy element nucleosynthesis. In addition age determinations, based upon long-lived radioactive nuclei abundances, can now be obtained. These stellar abundance determinations depend critically upon atomic data. Improved laboratory transition probabilities have been recently obtained for a number of elements. These new gf values have been used to greatly refine the abundances of neutron-capture elemental abundances in the solar photosphere and in very metal-poor Galactic halo stars. The newly determined stellar abundances are surprisingly consistent with a (relative) Solar System r-process pattern, and are also consistent with abundance predictions expected from such neutron-capture nucleosynthesis.

  1. Broad Band Properties of the BAT Selected AGN

    NASA Technical Reports Server (NTRS)

    Mushotzky, Richard; Winter, Lisa; Tueller, jack

    2008-01-01

    We will present the x-ray spectral properties of approximately 150 Burst Alert Telescope (BAT) selected active galactic nuclei (AGN) focusing on the issues of spectral complexity, x-ray absorption and its distribution and that contribution of sources to the x-ray background. If time permits we will also present the nature of the host galaxies of the AGN and their relationship to merger candidates.

  2. 3D atom microscopy in the presence of Doppler shift

    NASA Astrophysics Data System (ADS)

    Rahmatullah; Chuang, You-Lin; Lee, Ray-Kuang; Qamar, Sajid

    2018-03-01

    The interaction of hot atoms with laser fields produces a Doppler shift, which can severely affect the precise spatial measurement of an atom. We suggest an experimentally realizable scheme to address this issue in the three-dimensional position measurement of a single atom in vapors of rubidium atoms. A three-level Λ-type atom-field configuration is considered where a moving atom interacts with three orthogonal standing-wave laser fields and spatial information of the atom in 3D space is obtained via an upper-level population using a weak probe laser field. The atom moves with velocity v along the probe laser field, and due to the Doppler broadening the precision of the spatial information deteriorates significantly. It is found that via a microwave field, precision in the position measurement of a single hot rubidium atom can be attained, overcoming the limitation posed by the Doppler shift.

  3. Observations of CO2 in Comets C/2012 S1 ISON and C/2012 K1 PANSTARRS

    NASA Astrophysics Data System (ADS)

    McKay, Adam; Kelley, Michael; DiSanti, Michael; Cochran, Anita; Dello Russo, Neil; Lisse, Carey; Chanover, Nancy

    2013-10-01

    Comets have undergone very little thermal evolution in their lifetimes, resulting in a primitive composition. This primitive composition makes observations of comets very important tools for understanding the origin of the Solar System. The ices H2O, CO2, and CO are the primary ices present in cometary nuclei, and constraining their abundances has tremendous implications for the formation and evolutionary history of comets. Of these ices, H2O and CO can be observed from the ground, while CO2 cannot. A potentially effective tracer for CO2 in comets that is accessible from the ground is atomic oxygen. However, the relationship between these ices and atomic oxygen is only understood at a qualitative level. We propose to use Spitzer observations in IRAC's 4.5 micron band pass to observe the CO2 v3 band at 4.26 microns in comets C/2012 S1 ISON and C/2012 K1 PANSTARRS. These observations will be coordinated with observations of atomic oxygen obtained at Apache Point Observatory and McDonald Observatory and observations of H2O and CO at Keck and IRTF. These observations of H2O, CO2, and atomic oxygen in a cometary coma will increase our understanding of the link between these primary ices and atomic oxygen. With a complete understanding of the relationship between atomic oxygen and the primary ices on the nucleus, observations of atomic oxygen can serve as a powerful proxy for the production of CO2. In addition, ISON is the target of an extensive observing campaign led by NASA, and the proposed Spitzer observations fill a vital niche as the only observatory that can observe CO2 during both the near-perihelion time frame and significantly (months) after perihelion. Understanding the evolution of the CO2 abundance over the apparition is a key piece to understanding how the volatile compostion of the comet changes over the apparition.

  4. OH megamasers in high-luminosity IRAS galaxies

    NASA Technical Reports Server (NTRS)

    Mirabel, I. F.; Sanders, D. B.

    1987-01-01

    OH megamaser emission and H I and CO profiles from the distant infrared galaxies IRAS 10173 + 0828, III Zw 035, and Zw 475.056 are reported. The OH isotropic luminosities at 1667 MHz are 463, 534, and 6.6 solar luminosities, respectively. Far-infrared pumping efficiencies of the OH greater than 1 percent are found in IRAS 10173 + 0828 and III Zw 035. These two galaxies show anomalously large 1667/1665 MHz emission line ratios. OH megamasers reside in the nuclei of superluminous far-infrared galaxies that have a high content of molecular gas, high efficiency of star formation, and in some instances, a striking deficiency of atomic hydrogen.

  5. Geant4 Developments for the Radon Electric Dipole Moment Search at TRIUMF

    NASA Astrophysics Data System (ADS)

    Rand, E. T.; Bangay, J. C.; Bianco, L.; Dunlop, R.; Finlay, P.; Garrett, P. E.; Leach, K. G.; Phillips, A. A.; Sumithrarachchi, C. S.; Svensson, C. E.; Wong, J.

    2011-09-01

    An experiment is being developed at TRIUMF to search for a time-reversal violating electric dipole moment (EDM) in odd-A isotopes of Rn. Extensive simulations of the experiment are being performed with GEANT4 to study the backgrounds and sensitivity of the proposed measurement technique involving the detection of γ rays emitted following the β decay of polarized Rn nuclei. GEANT4 developments for the RnEDM experiment include both realistic modelling of the detector geometry and full tracking of the radioactive β, γ, internal conversion, and x-ray processes, including the γ-ray angular distributions essential for measuring an atomic EDM.

  6. Radiative transfer in scattering stochastic atmospheres

    NASA Astrophysics Data System (ADS)

    Silant'ev, N. A.; Alekseeva, G. A.; Novikov, V. V.

    2017-12-01

    Many stars, active galactic nuclei, accretion discs etc. are affected by the stochastic variations of temperature, turbulent gas motions, magnetic fields, number densities of atoms and dust grains. These stochastic variations influence on the extinction factors, Doppler widths of lines and so on. The presence of many reasons for fluctuations gives rise to Gaussian distribution of fluctuations. The usual models leave out of account the fluctuations. In many cases the consideration of fluctuations improves the coincidence of theoretical values with the observed data. The objective of this paper is the investigation of the influence of the number density fluctuations on the form of radiative transfer equations. We consider non-magnetized atmosphere in continuum.

  7. 53Cr NMR study of CuCrO2 multiferroic

    NASA Astrophysics Data System (ADS)

    Smol'nikov, A. G.; Ogloblichev, V. V.; Verkhovskii, S. V.; Mikhalev, K. N.; Yakubovskii, A. Yu.; Kumagai, K.; Furukawa, Y.; Sadykov, A. F.; Piskunov, Yu. V.; Gerashchenko, A. P.; Barilo, S. N.; Shiryaev, S. V.

    2015-11-01

    The magnetically ordered phase of the CuCrO2 single crystal has been studied by the nuclear magnetic resonance (NMR) method on 53Cr nuclei in the absence of an external magnetic field. The 53Cr NMR spectrum is observed in the frequency range νres = 61-66 MHz. The shape of the spectrum depends on the delay tdel between pulses in the pulse sequence τπ/2- t del-τπ- t del-echo. The spin-spin and spin-lattice relaxation times have been measured. Components of the electric field gradient, hyperfine fields, and the magnetic moment on chromium atoms have been estimated.

  8. Puzzling questions about excited superdeformed rotational bands of atomic nuclei are answered by the two-revolving-cluster model.

    PubMed Central

    Pauling, L

    1992-01-01

    The two-revolving-cluster model provides explanations of several questions about excited superdeformed bands: restriction to the lanthanons and the Hg-Tl-Pb region and to the smaller values of the neutron number for each element, truncation of the gamma-ray cascades, differences in shape of the lanthanon and Hg-Tl-Pb bands, alignment of quantified spins, and the existence of pairs of bands with nearly identical gamma-ray sequences. A previously unrecognized kind of pairing (intercalation of gamma-ray values) is also reported and a discussion is given of the values of electric quadrupole moments. PMID:11607327

  9. Laser ablated hydantoin: A high resolution rotational study.

    PubMed

    Alonso, Elena R; Kolesniková, Lucie; Alonso, José L

    2017-09-28

    Laser ablation techniques coupled with broadband and narrowband Fourier transform microwave spectroscopies have allowed the high resolution rotational study of solid hydantoin, an important target in astrochemistry as a possible precursor of glycine. The complicated hyperfine structure arising from the presence of two 14 N nuclei in non-equivalent positions has been resolved and interpreted in terms of the nuclear quadrupole coupling interactions. The results reported in this work provide a solid base for the interstellar searches of hydantoin in the astrophysical surveys. The values of the nuclear quadrupole coupling constants have been also discussed in terms of the electronic environment around the respective nitrogen atom.

  10. Collision for Li++He System. I. Potential Curves and Non-Adiabatic Coupling Matrix Elements

    NASA Astrophysics Data System (ADS)

    Yoshida, Junichi; O-Ohata, Kiyosi

    1984-02-01

    The potential curves and the non-adiabatic coupling matrix elements for the Li++He collision system were computed. The SCF molecular orbitals were constructed with the CGTO atomic bases centered on each nucleus and the center of mass of two nuclei. The SCF and CI calculations were done at various internuclear distances in the range of 0.1˜25.0 a.u. The potential energies and the wavefunctions were calculated with good approximation over whole internuclear distance. The non-adiabatic coupling matrix elements were calculated with the tentative method in which the ETF are approximately taken into account.

  11. HST update - Science amid setbacks

    NASA Astrophysics Data System (ADS)

    Fienberg, Richard T.

    1991-09-01

    Recent data obtained from the Hubble Space Telescope (HST) are presented that indicate that the mission of the beleagered telescope has reached a turning point. Among these observations is a spectrogram revealing the complex dynamic structure of the Beta Pictoris's gas disk, the Lyman-alpha lines from clouds of cool hydrogen atoms in the Milky Way, the UV spectrum of Chi Lupi, the images of Eta Carinae and the Homunculus nebula ejected by the star during the 1843 outburst, and the structure of energetic jets from active galactic nuclei. The paper discusses corrective measures planned by the NASA and Hubble project astronomers to restore the observatory to near-perfect health.

  12. Left right asymmetry of nuclear shadowing in charged current DIS

    NASA Astrophysics Data System (ADS)

    Fiore, R.; Zoller, V. R.

    2006-01-01

    We study the shadowing effect in highly asymmetric diffractive interactions of left- and right-handed W-bosons with atomic nuclei. The target nucleus is found to be quite transparent for the charmed-strange Fock component of the light-cone W+ in the helicity state λ = + 1 and rather opaque for the csbar dipole with λ = - 1. The shadowing correction to the structure function ΔxF3 = x F3νN - x F3νbarN extracted from νFe and νbar Fe data is shown to make up about 20% in the kinematical range of CCFR/NuTeV.

  13. Energy-range relations for hadrons in nuclear matter

    NASA Technical Reports Server (NTRS)

    Strugalski, Z.

    1985-01-01

    Range-energy relations for hadrons in nuclear matter exist similarly to the range-energy relations for charged particles in materials. When hadrons of GeV kinetic energies collide with atomic nuclei massive enough, events occur in which incident hadron is stopped completely inside the target nucleus without causing particle production - without pion production in particular. The stoppings are always accompanied by intensive emission of nucleons with kinetic energy from about 20 up to about 400 MeV. It was shown experimentally that the mean number of the emitted nucleons is a measure of the mean path in nuclear matter in nucleons on which the incident hadrons are stopped.

  14. Neutron displacement cross-sections for tantalum and tungsten at energies up to 1 GeV

    NASA Astrophysics Data System (ADS)

    Broeders, C. H. M.; Konobeyev, A. Yu.; Villagrasa, C.

    2005-06-01

    The neutron displacement cross-section has been evaluated for tantalum and tungsten at energies from 10 -5 eV up to 1 GeV. The nuclear optical model, the intranuclear cascade model combined with the pre-equilibrium and evaporation models were used for the calculations. The number of defects produced by recoil atoms nuclei in materials was calculated by the Norgett, Robinson, Torrens model and by the approach combining calculations using the binary collision approximation model and the results of the molecular dynamics simulation. The numerical calculations were done using the NJOY code, the ECIS96 code, the MCNPX code and the IOTA code.

  15. Hypercubane: DFT-based prediction of an Oh-symmetric double-shell hydrocarbon

    NASA Astrophysics Data System (ADS)

    Pichierri, Fabio

    2014-09-01

    Using density functional theory we design a molecular analog of the four-dimensional hypercube or tesseract which we called hypercubane. The title hydrocarbon (C40H24) is Oh-symmetric like cubane and is characterized by a double-shell architecture. The perfluorinated analog of hypercubane also is stable with a positive value of the electron affinity. Removal of the C8 core from hypercubane yields a hollowed Oh-symmetric hydrocarbon with enough room to host a single atom/ion guest. The resonances of the NMR-active 13C and 1H nuclei have been computed so as to assist the spectroscopic identification of the predicted molecules.

  16. Localized N, {lambda}, {sigma}, and {xi} single-particle potentials in finite nuclei calculated with SU{sub 6} quark-model baryon-baryon interactions

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kohno, M.; Fujiwara, Y.

    Localized single-particle potentials for all octet baryons, N, {lambda}, {sigma}, and {xi}, in finite nuclei, {sup 12}C, {sup 16}O, {sup 28}Si, {sup 40}Ca, {sup 56}Fe, and {sup 90}Zr, are calculated using the quark-model baryon-baryon interactions. G matrices evaluated in symmetric nuclear matter in the lowest order Brueckner theory (LOBT) are applied to finite nuclei in local density approximation. Nonlocal potentials are localized by a zero-momentum Wigner transformation. Empirical single-particle properties of the nucleon and the {lambda} hyperon in a nuclear medium have been known to be explained semiquantitatively in the LOBT framework. Attention is focused in the present consideration onmore » predictions for the {sigma} and {xi} hyperons. The unified description for the octet baryon-baryon interactions by the SU{sub 6} quark model enables us to obtain less ambiguous extrapolation to the S=-1 and S=-2 sectors based on the knowledge in the NN sector than other potential models. The {sigma} mean field is shown to be weakly attractive at the surface, but turns out to be repulsive inside, which is consistent with the experimental evidence. The {xi} hyperon s.p. potential is also attractive at the nuclear surface region, and inside it fluctuates around zero. Hence {xi} hypernuclear bound states are unlikely. We also evaluate energy shifts of the {sigma}{sup -} and {xi}{sup -} atomic levels in {sup 28}Si and {sup 56}Fe, using the calculated s.p. potentials.« less

  17. Irreversible barrier to the reprogramming of donor cells in cloning with mouse embryos and embryonic stem cells.

    PubMed

    Ono, Yukiko; Kono, Tomohiro

    2006-08-01

    Somatic cloning does not always result in ontogeny in mammals, and development is often associated with various abnormalities and embryo loss with a high frequency. This is considered to be due to aberrant gene expression resulting from epigenetic reprogramming errors. However, a fundamental question in this context is whether the developmental abnormalities reported to date are specific to somatic cloning. The aim of this study was to determine the stage of nuclear differentiation during development that leads to developmental abnormalities associated with embryo cloning. In order to address this issue, we reconstructed cloned embryos using four- and eight-cell embryos, morula embryos, inner cell mass (ICM) cells, and embryonic stem cells as donor nuclei and determined the occurrence of abnormalities such as developmental arrest and placentomegaly, which are common characteristics of all mouse somatic cell clones. The present analysis revealed that an acute decline in the full-term developmental competence of cloned embryos occurred with the use of four- and eight-cell donor nuclei (22.7% vs. 1.8%) in cases of standard embryo cloning and with morula and ICM donor nuclei (11.4% vs. 6.6%) in serial nuclear transfer. Histological observation showed abnormal differentiation and proliferation of trophoblastic giant cells in the placentae of cloned concepti derived from four-cell to ICM cell donor nuclei. Enlargement of placenta along with excessive proliferation of the spongiotrophoblast layer and glycogen cells was observed in the clones derived from morula embryos and ICM cells. These results revealed that irreversible epigenetic events had already started to occur at the four-cell stage. In addition, the expression of genes involved in placentomegaly is regulated at the blastocyst stage by irreversible epigenetic events, and it could not be reprogrammed by the fusion of nuclei with unfertilized oocytes. Hence, developmental abnormalities such as placentomegaly as well as embryo loss during development may occur even in cloned embryos reconstructed with nuclei from preimplantation-stage embryos, and these abnormalities are not specific to somatic cloning.

  18. Atomic Safety and Licensing Board Panel Biennial Report, Fiscal Years 1993--1994. Volume 6

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1995-08-01

    In Fiscal Year 1993, the Atomic Safety and Licensing Board Panel (``the Panel``) handled 30 proceedings. In Fiscal Year 1994, the Panel handled 36 proceedings. The cases addressed issues in the construction, operation, and maintenance of commercial nuclear power reactors and other activities requiring a license form the Nuclear Regulatory Commission. This report sets out the Panel`s caseload during the year and summarizes, highlight, and analyzes how the wide- ranging issues raised in those proceedings were addressed by the Panel`s judges and licensing boards.

  19. Fabrication of Nanolaminates with Ultrathin Nanolayers Using Atomic Layer Deposition: Nucleation & Growth Issues

    DTIC Science & Technology

    2009-02-01

    Tecnologia de Superficies y Materiales (SMCTSM), XXVII Congreso Nacional, Oaxaca, Oaxaca, Mexico, September 26, 2007. 26. "Atomic Layer Deposition of...Nanolaminates: Fabrication and Properties" (Plenary Lecture), Sociedad Mexicana de Ciencia y Tecnologia de Superficies y Materiales (SMCTSM), XXVII

  20. 77 FR 71454 - Notice of Atomic Safety And Licensing Board Reconstitution, Tennessee Valley Authority (Watts Bar...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-11-30

    ... accordance with the NRC E-Filing rule. See 10 CFR 2.302 et seq. Issued at Rockville, Maryland this 16th day of November 2012. E. Roy Hawkens, Chief Administrative Judge, Atomic Safety and Licensing Board Panel...

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