Detection of Gravitational Wave Emission by Supermassive Black Hole Binaries Through Tidal Disruption Flares

PubMed Central

Hayasaki, Kimitake; Loeb, Abraham

2016-01-01

Galaxy mergers produce supermassive black hole binaries, which emit gravitational waves prior to their coalescence. We perform three-dimensional hydrodynamic simulations to study the tidal disruption of stars by such a binary in the final centuries of its life. We find that the gas stream of the stellar debris moves chaotically in the binary potential and forms accretion disks around both black holes. The accretion light curve is modulated over the binary orbital period owing to relativistic beaming. This periodic signal allows to detect the decay of the binary orbit due to gravitational wave emission by observing two tidal disruption events that are separated by more than a decade. PMID:27767188

Population of Nuclei Via 7Li-Induced Binary Reactions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Clark, Rodney M.; Phair, Larry W.; Descovich, M.

2005-08-08

The authors have investigated the population of nuclei formed in binary reactions involving {sup 7}Li beams on targets of {sup 160}Gd and {sup 184}W. The {sup 7}Li + {sup 184}W data were taken in the first experiment using the LIBERACE Ge-array in combination with the STARS Si {Delta}E-E telescope system at the 88-Inch Cyclotron of the Lawrence Berkeley National Laboratory. By using the Wilczynski binary transfer model, in combination with a standard evaporation model, they are able to reproduce the experimental results. This is a useful method for predicting the population of neutron-rich heavy nuclei formed in binary reactions involvingmore » beams of weakly bound nuclei formed in binary reactions involving beams of weakly bound nuclei and will be of use in future spectroscopic studies.« less

Binary Inspiral in Quadratic Gravity

NASA Astrophysics Data System (ADS)

Yagi, Kent

2015-01-01

Quadratic gravity is a general class of quantum-gravity-inspired theories, where the Einstein-Hilbert action is extended through the addition of all terms quadratic in the curvature tensor coupled to a scalar field. In this article, we focus on the scalar Gauss- Bonnet (sGB) theory and consider the black hole binary inspiral in this theory. By applying the post-Newtonian (PN) formalism, we found that there is a scalar dipole radiation which leads to -1PN correction in the energy flux relative to gravitational radiation in general relativity. From the orbital decay rate of a low-mass X-ray binary A0600-20, we obtain the bound that is six orders of magnitude stronger than the current solar system bound. Furthermore, we show that the excess in the orbital decay rate of XTE J1118+480 can be explained by the scalar radiation in sGB theory.

Self-organization in a system of binary strings with spatial interactions

NASA Astrophysics Data System (ADS)

Banzhaf, W.; Dittrich, P.; Eller, B.

1999-01-01

We consider an artificial reaction system whose components are binary strings. Upon encounter, two binary strings produce a third string which competes for storage space with the originators. String types or species can only survive when produced in sufficient numbers. Spatial interactions through introduction of a topology and rules for distance-dependent reactions are discussed. We observe various kinds of survival strategies of binary strings.

A diagrammatic formulation of the kinetic theory of fluctuations in equilibrium classical fluids. VI. Binary collision approximations for the memory function for self-correlation functions

NASA Astrophysics Data System (ADS)

Noah-Vanhoucke, Joyce E.; Andersen, Hans C.

2007-08-01

We use computer simulation results for a dense Lennard-Jones fluid for a range of temperatures to test the accuracy of various binary collision approximations for the memory function for density fluctuations in liquids. The approximations tested include the moderate density approximation of the generalized Boltzmann-Enskog memory function (MGBE) of Mazenko and Yip [Statistical Mechanics. Part B. Time-Dependent Processes, edited by B. J. Berne (Plenum, New York, 1977)], the binary collision approximation (BCA) and the short time approximation (STA) of Ranganathan and Andersen [J. Chem. Phys. 121, 1243 (2004); J. Phys. Chem. 109, 21437 (2005)] and various other approximations we derived by using diagrammatic methods. The tests are of two types. The first is a comparison of the correlation functions predicted by each approximate memory function with the simulation results, especially for the self-longitudinal current correlation (SLCC) function. The second is a direct comparison of each approximate memory function with a memory function numerically extracted from the correlation function data. The MGBE memory function is accurate at short times but decays to zero too slowly and gives a poor description of the correlation function at intermediate times. The BCA is exact at zero time, but it predicts a correlation function that diverges at long times. The STA gives a reasonable description of the SLCC but does not predict the correct temperature dependence of the negative dip in the function that is associated with caging at low temperatures. None of the other binary collision approximations is a systematic improvement on the STA. The extracted memory functions have a rapidly decaying short time part, much like the STA, and a much smaller, more slowly decaying part of the type predicted by a mode coupling theory. Theories that use mode coupling commonly include a binary collision term in the memory function but do not discuss in detail the nature of that term. It is clear from the present work that the short time part of the memory function has a behavior associated with brief binary repulsive collisions, such as those described by the STA. Collisions that include attractive as well as repulsive interactions, such as those of the MGBE, have a much longer duration, and theories that include them have memory functions that decay to zero much too slowly to provide a good first approximation of the correlation function. This leads us to speculate that the memory function for density fluctuations can be usefully regarded as a sum of at least three parts: a contribution from repulsive binary collisions (the STA or something similar to it), another short time part that is related to all the other interactions (but whose nature is not understood), and a longer time slowly decaying part that describes caging (of the type predicted by the mode coupling theory).

Detectability of compact binary merger macronovae

NASA Astrophysics Data System (ADS)

Rosswog, S.; Feindt, U.; Korobkin, O.; Wu, M.-R.; Sollerman, J.; Goobar, A.; Martinez-Pinedo, G.

2017-05-01

We study the optical and near-infrared luminosities and detectability of radioactively powered electromagnetic transients (‘macronovae’) occuring in the aftermath of binary neutron star and neutron star black hole mergers. We explore the transients that result from the dynamic ejecta and those from different types of wind outflows. Based on full nuclear network simulations we calculate the resulting light curves in different wavelength bands. We scrutinize the robustness of the results by comparing (a) two different nuclear reaction networks and (b) two macronova models. We explore in particular how sensitive the results are to the production of α-decaying trans-lead nuclei. We compare two frequently used mass models: the finite-range Droplet model (FRDM) and the nuclear mass model of Duflo and Zuker (DZ31). We find that the abundance of α-decaying trans-lead nuclei has a significant impact on the observability of the resulting macronovae. For example, the DZ31 model yields considerably larger abundances resulting in larger heating rates and thermalization efficiencies and therefore predicts substantially brighter macronova transients. We find that the dynamic ejecta from NSNS models can reach peak K-band magnitudes in excess of  -15 while those from NSBH cases can reach beyond  -16. Similar values can be reached by some of our wind models. Several of our models (both wind and dynamic ejecta) yield properties that are similar to the transient that was observed in the aftermath of the short GRB 130603B. We further explore the expected macronova detection frequencies for current and future instruments such as VISTA, ZTF and LSST.

Brown Dwarf Companion Frequencies and Dynamical Interactions

NASA Astrophysics Data System (ADS)

Sterzik, Michael F.; Durisen, Richard H.

2003-06-01

Numerical simulations are used to explore how gravitational interactions within young multiple star systems may determine the binary properties of brown dwarfs. We compare different scenarios for cluster formation and decay and find that brown dwarf binaries, although possible, generally have a low frequency. We also discuss the frequencies of brown dwarf companions to normal stars expected from these models.

On the frequency of close binary systems among very low-mass stars and brown dwarfs

NASA Astrophysics Data System (ADS)

Maxted, P. F. L.; Jeffries, R. D.

2005-09-01

We have used Monte Carlo simulation techniques and published radial velocity surveys to constrain the frequency of very low-mass star (VLMS) and brown dwarf (BD) binary systems and their separation (a) distribution. Gaussian models for the separation distribution with a peak at a= 4au and 0.6 <=σlog(a/au)<= 1.0, correctly predict the number of observed binaries, yielding a close (a < 2.6au) binary frequency of 17-30 per cent and an overall VLMS/BD binary frequency of 32-45 per cent. We find that the available N-body models of VLMS/BD formation from dynamically decaying protostellar multiple systems are excluded at >99 per cent confidence because they predict too few close binary VLMS/BDs. The large number of close binaries and high overall binary frequency are also very inconsistent with recent smoothed particle hydrodynamical modelling and argue against a dynamical origin for VLMS/BDs.

Close binary systems among very low-mass stars and brown dwarfs

NASA Astrophysics Data System (ADS)

Jeffries, R. D.; Maxted, P. F. L.

2005-12-01

Using Monte Carlo simulations and published radial velocity surveys we have constrained the frequency and separation (a) distribution of very low-mass star (VLM) and brown dwarf (BD) binary systems. We find that simple Gaussian extensions of the observed wide binary distribution, with a peak at 4 AU and 0.6<\\sigma_{\\log(a/AU)}<1.0, correctly reproduce the observed number of close binary systems, implying a close (a<2.6 AU) binary frequency of 17-30 % and overall frequency of 32-45 %. N-body models of the dynamical decay of unstable protostellar multiple systems are excluded with high confidence because they do not produce enough close binary VLMs/BDs. The large number of close binaries and high overall binary frequency are also completely inconsistent with published smoothed particle hydrodynamical modelling and argue against a dynamical origin for VLMs/BDs.

Reactivity of bromoalkanes in reactions of coordinated molecular decay

NASA Astrophysics Data System (ADS)

Pokidova, T. S.; Denisov, E. T.

2016-09-01

The results from experiments on reactions of the coordinated molecular decay of RBr bromoalkanes on olefin and HBr are analyzed using the model of intersecting parabolas (MIP). Kinetic parameters within the MIP are calculated from the experimental data, enabling calculation of the activation energies ( E) and rate constants ( k) of such reactions, based on the enthalphy of the reaction and the MIP algorithms. The factors affecting the E of the RBr decay reaction are established: the enthalphy of the reaction, triplet repulsion, the energy of radical R• stabilization, the presence of a π bond adjacent to the reaction center, and the dipole-dipole interaction of polar groups. The energy spectrum of the partial energies of activation is constructed for the reaction of coordinated molecular decay of RBr, and the E and k of inverse addition reactions are evaluated.

Orbital Decay in Binaries with Evolved Stars

NASA Astrophysics Data System (ADS)

Sun, Meng; Arras, Phil; Weinberg, Nevin N.; Troup, Nicholas; Majewski, Steven R.

2018-01-01

Two mechanisms are often invoked to explain tidal friction in binary systems. The ``dynamical tide” is the resonant excitation of internal gravity waves by the tide, and their subsequent damping by nonlinear fluid processes or thermal diffusion. The ``equilibrium tide” refers to non-resonant excitation of fluid motion in the star’s convection zone, with damping by interaction with the turbulent eddies. There have been numerous studies of these processes in main sequence stars, but less so on the subgiant and red giant branches. Motivated by the newly discovered close binary systems in the Apache Point Observatory Galactic Evolution Experiment (APOGEE-1), we have performed calculations of both the dynamical and equilibrium tide processes for stars over a range of mass as the star’s cease core hydrogen burning and evolve to shell burning. Even for stars which had a radiative core on the main sequence, the dynamical tide may have very large amplitude in the newly radiative core in post-main sequence, giving rise to wave breaking. The resulting large dynamical tide dissipation rate is compared to the equilibrium tide, and the range of secondary masses and orbital periods over which rapid orbital decay may occur will be discussed, as well as applications to close APOGEE binaries.

Hadronic model for the non-thermal radiation from the binary system AR Scorpii

NASA Astrophysics Data System (ADS)

Bednarek, W.

2018-05-01

AR Scorpii is a close binary system containing a rotation powered white dwarf and a low-mass M type companion star. This system shows non-thermal emission extending up to the X-ray energy range. We consider hybrid (lepto-hadronic) and pure hadronic models for the high energy non-thermal processes in this binary system. Relativistic electrons and hadrons are assumed to be accelerated in a strongly magnetised, turbulent region formed in collision of a rotating white dwarf magnetosphere and a magnetosphere/dense atmosphere of the M-dwarf star. We propose that the non-thermal X-ray emission is produced either by the primary electrons or the secondary e± pairs from decay of charged pions created in collisions of hadrons with the companion star atmosphere. We show that the accompanying γ-ray emission from decay of neutral pions, which are produced by these same protons, is expected to be on the detectability level of the present and/or the future satellite and Cherenkov telescopes. The γ-ray observations of the binary system AR Sco should allow us to constrain the efficiency of hadron and electron acceleration and also the details of the radiation processes.

Does mass accretion lead to field decay in neutron stars

NASA Technical Reports Server (NTRS)

Shibazaki, N.; Murakami, T.; Shaham, Jacob; Nomoto, K.

1989-01-01

The recent discovery of cyclotron lines from gamma-ray bursts indicates that the strong magnetic fields of isolated neutron stars might not decay. The possible inverse correlation between the strength of the magnetic field and the mass accreted by the neutron star suggests that mass accretion itself may lead to the decay of the magnetic field. The spin and magnetic field evolution of the neutron star was calculated under the hypothesis of the accretion-induced field decay. It is shown that the calculated results are consistent with the observations of binary and millisecond radio pulsars.

Trojan horse particle invariance studied with the {sup 6}Li(d,{alpha}){sup 4}He and {sup 7}Li(p,{alpha}){sup 4}He reactions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pizzone, R. G.; Spitaleri, C.; Lamia, L.

2011-04-15

The Trojan horse nucleus invariance for the binary reaction cross section extracted from the Trojan horse reaction was tested using the quasifree {sup 3}He({sup 6}Li,{alpha}{alpha})H and {sup 3}He({sup 7}Li,{alpha}{alpha}){sup 2}H reactions. The cross sections for the {sup 6}Li(d,{alpha}){sup 4}He and {sup 7}Li(p,{alpha}){sup 4}He binary processes were extracted in the framework of the plane wave approximation. They are compared with direct behaviors as well as with cross sections extracted from previous indirect investigations of the same binary reactions using deuteron as the Trojan horse nucleus instead of {sup 3}He. The very good agreement confirms the applicability of the plane wave approximationmore » which suggests the independence of the binary indirect cross section on the chosen Trojan horse nucleus, at least for the investigated cases.« less

Are Binary Separations related to their System Mass?

NASA Astrophysics Data System (ADS)

Sterzik, M. F.; Durisen, R. H.

2004-08-01

We compile most recent multiplicity fractions and binary separation distributions for different primary masses, including very low-mass and brown dwarf primaries, and compare them with dynamical decay models of small-N clusters. The model predictions are based on detailed numerical calculations of the internal cluster dynamics, as well as on Monte-Carlo methods. Both observations and models reflect the same trends: (1) The multiplicity fraction is an increasing function of the primary mass. (2) The mean binary separations are increasing with the system mass in the sense that very low-mass binaries have average separations around ≈ 4AU, while the binary separation distribution for solar-type primaries peaks at ≈ 40AU. M-type binary systems apparently preferentially populate intermediate separations. Similar specific energy at the time of cluster formation for all cluster masses can possibly explain this trend.

Beta-Decay Rates for Exotic Nuclei and R-Process Nucleosynthesis

NASA Astrophysics Data System (ADS)

Suzuki, Toshio; Yoshida, Takashi; Wanajo, Shinya; Kajino, Toshitaka; Otsuka, Takaharu

Beta-decay rates for exotic nuclei at N = 126 relevant to r-process nucleosynthesis are studied by shell-model calculations. The half-lives obtained are used to study r-process nucleosynthesis in core-collapse supernova explosions and binary neutron star mergers. The element abundances are obtained up to the third peak as well as beyond the peak region up to uranium.

Coevolution of Binaries and Circumbinary Gaseous Disks

NASA Astrophysics Data System (ADS)

Fleming, David; Quinn, Thomas R.

2018-04-01

The recent discoveries of circumbinary planets by Kepler raise questions for contemporary planet formation models. Understanding how these planets form requires characterizing their formation environment, the circumbinary protoplanetary disk, and how the disk and binary interact. The central binary excites resonances in the surrounding protoplanetary disk that drive evolution in both the binary orbital elements and in the disk. To probe how these interactions impact both binary eccentricity and disk structure evolution, we ran N-body smooth particle hydrodynamics (SPH) simulations of gaseous protoplanetary disks surrounding binaries based on Kepler 38 for 10^4 binary orbital periods for several initial binary eccentricities. We find that nearly circular binaries weakly couple to the disk via a parametric instability and excite disk eccentricity growth. Eccentric binaries strongly couple to the disk causing eccentricity growth for both the disk and binary. Disks around sufficiently eccentric binaries strongly couple to the disk and develop an m = 1 spiral wave launched from the 1:3 eccentric outer Lindblad resonance (EOLR). This wave corresponds to an alignment of gas particle longitude of periastrons. We find that in all simulations, the binary semi-major axis decays due to dissipation from the viscous disk.

Dynamics of phase separation of binary fluids

NASA Technical Reports Server (NTRS)

Ma, Wen-Jong; Maritan, Amos; Banavar, Jayanth R.; Koplik, Joel

1992-01-01

The results of molecular-dynamics studies of surface-tension-dominated spinodal decomposition of initially well-mixed binary fluids in the absence and presence of gravity are presented. The growth exponent for the domain size and the decay exponent of the potential energy of interaction between the two species with time are found to be 0.6 +/- 0.1, inconsistent with scaling arguments based on dimensional analysis.

Aligning Metabolic Pathways Exploiting Binary Relation of Reactions.

PubMed

Huang, Yiran; Zhong, Cheng; Lin, Hai Xiang; Huang, Jing

2016-01-01

Metabolic pathway alignment has been widely used to find one-to-one and/or one-to-many reaction mappings to identify the alternative pathways that have similar functions through different sets of reactions, which has important applications in reconstructing phylogeny and understanding metabolic functions. The existing alignment methods exhaustively search reaction sets, which may become infeasible for large pathways. To address this problem, we present an effective alignment method for accurately extracting reaction mappings between two metabolic pathways. We show that connected relation between reactions can be formalized as binary relation of reactions in metabolic pathways, and the multiplications of zero-one matrices for binary relations of reactions can be accomplished in finite steps. By utilizing the multiplications of zero-one matrices for binary relation of reactions, we efficiently obtain reaction sets in a small number of steps without exhaustive search, and accurately uncover biologically relevant reaction mappings. Furthermore, we introduce a measure of topological similarity of nodes (reactions) by comparing the structural similarity of the k-neighborhood subgraphs of the nodes in aligning metabolic pathways. We employ this similarity metric to improve the accuracy of the alignments. The experimental results on the KEGG database show that when compared with other state-of-the-art methods, in most cases, our method obtains better performance in the node correctness and edge correctness, and the number of the edges of the largest common connected subgraph for one-to-one reaction mappings, and the number of correct one-to-many reaction mappings. Our method is scalable in finding more reaction mappings with better biological relevance in large metabolic pathways.

Development of a Monte Carlo code for the data analysis of the 18F(p,α)15O reaction at astrophysical energies

NASA Astrophysics Data System (ADS)

Caruso, A.; Cherubini, S.; Spitaleri, C.; Crucillà, V.; Gulino, M.; La Cognata, M.; Lamia, L.; Rapisarda, G.; Romano, S.; Sergi, ML.; Kubono, S.; Yamaguchi, H.; Hayakawa, S.; Wakabayashi, Y.; Iwasa, N.; Kato, S.; Komatsubara, T.; Teranishi, T.; Coc, A.; Hammache, F.; de Séréville, N.

2015-02-01

Novae are astrophysical events (violent explosion) occurring in close binary systems consisting of a white dwarf and a main-sequence star or a star in a more advanced stage of evolution. They are called "narrow systems" because the two components interact with each other: there is a process of mass exchange with resulting in the transfer of matter from the companion star to the white dwarf, leading to the formation of this last of the so-called accretion disk, rich mainly of hydrogen. Over time, more and more material accumulates until the pressure and the temperature reached are sufficient to trigger nuclear fusion reactions, rapidly converting a large part of the hydrogen into heavier elements. The products of "hot hydrogen burning" are then placed in the interstellar medium as a result of violent explosions. Studies on the element abundances observed in these events can provide important information about the stages of evolution stellar. During the outbursts of novae some radioactive isotopes are synthesized: in particular, the decay of short-lived nuclei such as 13N and 18F with subsequent emission of gamma radiation energy below 511 keV. The gamma rays from products electron-positron annihilation of positrons emitted in the decay of 18F are the most abundant and the first observable as soon as the atmosphere of the nova starts to become transparent to gamma radiation. Hence the importance of the study of nuclear reactions that lead both to the formation and to the destruction of 18F . Among these, the 18F(p,α)15O reaction is one of the main channels of destruction. This reaction was then studied at energies of astrophysical interest. The experiment done at Riken, Japan, has as its objective the study of the 18F(p,α)15O reaction, using a beam of 18F produced at CRIB, to derive important information about the phenomenon of novae. In this paper we present the experimental technique and the Monte Carlo code developed to be used in the data analysis process.

Strong binary pulsar constraints on Lorentz violation in gravity.

PubMed

Yagi, Kent; Blas, Diego; Yunes, Nicolás; Barausse, Enrico

2014-04-25

Binary pulsars are excellent laboratories to test the building blocks of Einstein's theory of general relativity. One of these is Lorentz symmetry, which states that physical phenomena appear the same for all inertially moving observers. We study the effect of violations of Lorentz symmetry in the orbital evolution of binary pulsars and find that it induces a much more rapid decay of the binary's orbital period due to the emission of dipolar radiation. The absence of such behavior in recent observations allows us to place the most stringent constraints on Lorentz violation in gravity, thus verifying one of the cornerstones of Einstein's theory much more accurately than any previous gravitational observation.

Analysis of decay chains of superheavy nuclei produced in the 249Bk+48Ca and 243Am+48Ca reactions

NASA Astrophysics Data System (ADS)

Zlokazov, V. B.; Utyonkov, V. K.

2017-07-01

The analysis of decay chains starting at superheavy nuclei 293Ts and 289Mc is presented. The spectroscopic properties of nuclei identified during the experiments using the 249Bk+48Ca and 243Am+48Ca reactions studied at the gas-filled separators DGFRS, TASCA and BGS are considered. We present the analysis of decay data using widely adopted statistical methods and applying them to the short decay chains of parent odd-Z nuclei. We find out that the recently suggested method of analyzing decay chains by Forsberg et al may lead to questionable conclusions when applied for the analysis of radioactive decays. Our discussion demonstrates reasonable congruence of α-particle energies and decay times of nuclei assigned to isotopes 289Mc, 285Nh and 281Rg observed in both reactions.

Accretion Disk Outflows from Compact Object Mergers

NASA Astrophysics Data System (ADS)

Metzger, Brian

Nuclear reactions play a key role in the accretion disks and outflows associated with the merger of binary compact objects and the central engines of gamma-ray bursts and supernovae. The proposed research program will investigate the impact of nucleosynthesis on these events and their observable signatures by means of analytic calculations and numerical simulations. One focus of this research is rapid accretion following the tidal disruption of a white dwarf (WD) by a neutron star (NS) or black hole (BH) binary companion. Tidal disruption shreds the WD into a massive torus composed of C, O, and/or He, which undergoes nuclear reactions and burns to increasingly heavier elements as it flows to smaller radii towards the central compact object. The nuclear energy so released is comparable to that released gravitationally, suggesting that burning could drastically alter the structure and stability of the accretion flow. Axisymmetric hydrodynamic simulations of the evolution of the torus including nuclear burning will be performed to explore issues such as the mass budget of the flow (accretion vs. outflows) and its thermal stability (steady burning and accretion vs. runaway explosion). The mass, velocity, and composition of outflows from the disk will be used in separate radiative transfer calculations to predict the lightcurves and spectra of the 56Ni-decay powered optical transients from WD-NS/WD-BH mergers. The possible connection of such events to recently discovered classes of sub-luminous Type I supernovae will be assessed. The coalescence of NS-NS/NS-BH binaries also results in the formation of a massive torus surrounding a central compact object. Three-dimensional magnetohydrodynamic simulations of the long-term evolution of such accretion disks will be performed, which for the first time follow the effects of weak interactions and the nuclear energy released by Helium recombination. The nucleosynthetic yield of disk outflows will be calculated using a detailed nuclear reaction network along characteristic Lagrangian trajectories. Results of these calculations will be used to (1) reassess NS-NS/NS-BH mergers as an astrophysical source of heavy r-process nuclei; and (2) calculate the light curves of the optical transients (`kilonovae') powered by the radioactive decay. Separate work will assess the effects that neutrino irradiation from a long-lived neutron star remnant has on the electron fraction of the disk outflows. The strong contrast between the opacities of proton- and neutron-rich matter imply that the presence and lifetime of such a remnant could be imprinted on the kilonova emission. Our investigation sheds light on the central engines of GRBs and other high-energy transients and hence is relevant to NASA's Swift, MAXI, and Fermi missions. Our results will also impact the interpretation of future observations of supernovae and their galactic environments with the Hubble Space Telescope (HST). Our results will also impact follow-up observations of kilonovae, maximizing the impact of HST to constrain the key open questions such as the progenitors of gamma-ray bursts and the origin of r-process nuclei.

Population of Nuclei Via 7Li-Induced Binary Reactions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Clark, R M; Phair, L W; Descovich, M

2005-08-09

The authors have investigated the population of nuclei formed in binary reactions involving {sup 7}Li beams on targets of {sup 160}Gd and {sup 184}W. The {sup 7}Li + {sup 184}W data were taken in the first experiment using the LIBERACE Ge-array in combination with the STARS Si {Delta}E-E telescope system at the 88-Inch Cyclotron of the Lawrence Berkeley National Laboratory. By using the Wilczynski binary transfer model, in combination with a standard evaporation model, they are able to reproduce the experimental results. This is a useful method for predicting the population of neutron-rich heavy nuclei formed in binary reactions involvingmore » beams of weakly bound nuclei and will be of use in future spectroscopic studies.« less

Measuring tides and binary parameters from gravitational wave data and eclipsing timings of detached white dwarf binaries

DOE Office of Scientific and Technical Information (OSTI.GOV)

Shah, Sweta; Nelemans, Gijs, E-mail: s.shah@astro.ru.nl

The discovery of the most compact detached white dwarf (WD) binary SDSS J065133.33+284423.3 has been discussed in terms of probing the tidal effects in WDs. This system is also a verification source for the space-based gravitational wave (GW) detector, eLISA, or the evolved Laser Interferometer Space Antenna, which will observe short-period compact Galactic binaries with P {sub orb} ≲ 5 hr. We address the prospects of performing tidal studies using eLISA binaries by showing the fractional uncertainties in the orbital decay rate, f-dot , and the rate of that decay, f{sup ¨} expected from both the GW and electromagnetic (EM)more » data for some of the high-f binaries. We find that f-dot and f{sup ¨} can be measured using GW data only for the most massive WD binaries observed at high frequencies. From timing the eclipses for ∼10 yr, we find that f-dot can be known to ∼0.1% for J0651. We find that from GW data alone, measuring the effects of tides in binaries is (almost) impossible. We also investigate the improvement in the knowledge of the binary parameters by combining the GW amplitude and inclination with EM data with and without f-dot . In our previous work, we found that EM data on distance constrained the 2σ uncertainty in chirp mass to 15%-25% whereas adding f-dot reduces it to 0.11%. EM data on f-dot also constrain the 2σ uncertainty in distance to 35%-19%. EM data on primary mass constrain the secondary mass m {sub 2} to factors of two to ∼40% whereas adding f-dot reduces this to 25%. Finally, using single-line spectroscopic data constrains 2σ uncertainties in both the m {sub 2}, d to factors of two to ∼40%. Adding EM data on f-dot reduces these 2σ uncertainties to ≤25% and 6%-19%, respectively. Thus we find that EM measurements of f-dot and radial velocity are valuable in constraining eLISA binary parameters.« less

Dynamical tides in highly eccentric binaries: chaos, dissipation, and quasi-steady state

NASA Astrophysics Data System (ADS)

Vick, Michelle; Lai, Dong

2018-05-01

Highly eccentric binary systems appear in many astrophysical contexts, ranging from tidal capture in dense star clusters, precursors of stellar disruption by massive black holes, to high-eccentricity migration of giant planets. In a highly eccentric binary, the tidal potential of one body can excite oscillatory modes in the other during a pericentre passage, resulting in energy exchange between the modes and the binary orbit. These modes exhibit one of three behaviours over multiple passages: low-amplitude oscillations, large-amplitude oscillations corresponding to a resonance between the orbital frequency and the mode frequency, and chaotic growth, with the mode energy reaching a level comparable to the orbital binding energy. We study these phenomena with an iterative map that includes mode dissipation, fully exploring how the mode evolution depends on the orbital and mode properties of the system. The dissipation of mode energy drives the system towards a quasi-steady state, with gradual orbital decay punctuated by resonances. We quantify the quasi-steady state and the long-term evolution of the system. A newly captured star around a black hole can experience significant orbital decay and heating due to the chaotic growth of the mode amplitude and dissipation. A giant planet pushed into a high-eccentricity orbit may experience a similar effect and become a hot or warm Jupiter.

Monodispersed porous flowerlike PtAu nanocrystals as effective electrocatalysts for ethanol oxidation

NASA Astrophysics Data System (ADS)

Li, Shumin; Xu, Hui; Xiong, Zhiping; Zhang, Ke; Wang, Caiqin; Yan, Bo; Guo, Jun; Du, Yukou

2017-11-01

Designing and tuning the bimetallic nanoparticles with desirable morphology and structure can embody them with greatly enhanced electrocatalytic activity and stability towards liquid fuel oxidation. We herein reported a facile one-pot method for the controlled synthesis of monodispersed binary PtAu nanoflowers with abundant exposed surface area. Owing to its fantastic structure, synergistic and electronic effect, such as-prepared PtAu nanoflowers exhibited outstandingly high electrocatalytic activity with the mass activity of 6482 mA mg-1 towards ethanol oxidation, which is 28.3 times higher than that of commercial Pt/C (227 mA mg-1). More interesting, the present PtAu nanoflower catalysts are more stable for the ethanol oxidation reaction in the alkaline with lower current density decay and retained a much higher current density after successive CVs of 500 cycles than that of commercial Pt/C. This work may open a new way for maximizing the catalytic performance of electrocatalysts towards ethanol oxidation by synthesizing shape-controlled alloy nanoparticles with more surface active sites to enhance the performances of direct fuel cells reaction, chemical conversion, and beyond.

Improved Limit on Direct α Decay of the Hoyle State

NASA Astrophysics Data System (ADS)

Kirsebom, O. S.; Alcorta, M.; Borge, M. J. G.; Cubero, M.; Diget, C. Aa.; Fraile, L. M.; Fulton, B. R.; Fynbo, H. O. U.; Galaviz, D.; Jonson, B.; Madurga, M.; Nilsson, T.; Nyman, G.; Riisager, K.; Tengblad, O.; Turrión, M.

2012-05-01

The current evaluation of the triple-α reaction rate assumes that the α decay of the 7.65 MeV, 0+ state in C12, commonly known as the Hoyle state, proceeds sequentially via the ground state of Be8. This assumption is challenged by the recent identification of two direct α-decay branches with a combined branching ratio of 17(5)%. If correct, this would imply a corresponding reduction in the triple-α reaction rate with important astrophysical consequences. We have used the B11(He3,d) reaction to populate the Hoyle state and measured the decay to three α particles in complete kinematics. We find no evidence for direct α-decay branches, and hence our data do not support a revision of the triple-α reaction rate. We obtain an upper limit of 5×10-3 on the direct α decay of the Hoyle state at 95% C.L., which is 1 order of magnitude better than a previous upper limit.

Binary Black Hole Mergers from Planet-like Migrations.

PubMed

Gould; Rix

2000-03-20

If supermassive black holes (BHs) are generically present in galaxy centers, and if galaxies are built up through hierarchical merging, BH binaries are at least temporary features of most galactic bulges. Observations suggest, however, that binary BHs are rare, pointing toward a binary lifetime far shorter than the Hubble time. We show that, almost regardless of the detailed mechanism, all stellar dynamical processes are too slow in reducing the orbital separation once orbital velocities in the binary exceed the virial velocity of the system. We propose that a massive gas disk surrounding a BH binary can effect its merger rapidly, in a scenario analogous to the orbital decay of super-Jovian planets due to a proto-planetary disk. As in the case of planets, gas accretion onto the secondary (here a supermassive BH) is integrally connected with its inward migration. Such accretion would give rise to quasar activity. BH binary mergers could therefore be responsible for many or most quasars.

Meson Production and Decays with WASA at COSY

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schadmand, Susan

2011-10-21

The WASA-at-COSY physics program focuses on light meson decays where rare decays are used to scrutinize symmetries and symmetry breaking. The structure of hadrons is probed with transition form factors and hadron spectroscopy while hadron dynamics is studied via reaction dynamics and few body reactions.

Partial Accretion in the Propeller Stage of Low-mass X-Ray Binary Aql X-1

NASA Astrophysics Data System (ADS)

Güngör, C.; Ekşi, K. Y.; Göğüş, E.; Güver, T.

2017-10-01

Aql X-1 is one of the most prolific low-mass X-ray binary transients (LMXBTs) showing outbursts almost annually. We present the results of our spectral analyses of Rossi X-Ray Timing Explorer/proportional counter-array observations of the 2000 and 2011 outbursts. We investigate the spectral changes related to the changing disk-magnetosphere interaction modes of Aql X-1. The X-ray light curves of the outbursts of LMXBTs typically show phases of fast rise and exponential decay. The decay phase shows a “knee” where the flux goes from the slow-decay to the rapid-decay stage. We assume that the rapid decay corresponds to a weak propeller stage at which a fraction of the inflowing matter in the disk accretes onto the star. We introduce a novel method for inferring, from the light curve, the fraction of the inflowing matter in the disk that accretes onto the neutron star depending on the fastness parameter. We determine the fastness parameter range within which the transition from the accretion to the partial propeller stage is realized. This fastness parameter range is a measure of the scale height of the disk in units of the inner disk radius. We applied the method to a sample of outbursts of Aql X-1 with different maximum flux and duration times. We show that different outbursts with different maximum luminosity and duration follow a similar path in the parameter space of accreted/inflowing mass flux fraction versus fastness parameter.

NuSTAR and XMM-Newton Observations of the 2015 Outburst Decay of GX 339-4

DOE Office of Scientific and Technical Information (OSTI.GOV)

Stiele, H.; Kong, A. K. H., E-mail: hstiele@mx.nthu.edu.tw

The extent of the accretion disk in the low/hard state of stellar mass black hole X-ray binaries remains an open question. There is some evidence suggesting that the inner accretion disk is truncated and replaced by a hot flow, while the detection of relativistic broadened iron emission lines seems to require an accretion disk extending fully to the innermost stable circular orbit. We present comprehensive spectral and timing analyses of six Nuclear Spectroscopic Telescope Array and XMM-Newton observations of GX 339–4 taken during outburst decay in the autumn of 2015. Using a spectral model consisting of a thermal accretion disk,more » Comptonized emission, and a relativistic reflection component, we obtain a decreasing photon index, consistent with an X-ray binary during outburst decay. Although we observe a discrepancy in the inner radius of the accretion disk and that of the reflector, which can be attributed to the different underlying assumptions in each model, both model components indicate a truncated accretion disk that resiles with decreasing luminosity. The evolution of the characteristic frequency in Fourier power spectra and their missing energy dependence support the interpretation of a truncated and evolving disk in the hard state. The XMM-Newton data set allowed us to study, for the first time, the evolution of the covariance spectra and ratio during outburst decay. The covariance ratio increases and steeps during outburst decay, consistent with increased disk instabilities.« less

Double core evolution. 7: The infall of a neutron star through the envelope of its massive star companion

NASA Technical Reports Server (NTRS)

Terman, James L.; Taam, Ronald E.; Hernquist, Lars

1995-01-01

Binary systems with properties similar to those of high-mass X-ray binaries are evolved through the common envelope phase. Three-dimensional simulations show that the timescale of the infall phase of the neutron star depends upon the evolutionary state of its massive companion. We find that tidal torques more effectively accelerate common envelope evolution for companions in their late core helium-burning stage and that the infall phase is rapid (approximately several initial orbital periods). For less evolved companions the decay of the orbit is longer; however, once the neutron star is deeply embedded within the companion's envelope the timescale for orbital decay decreases rapidly. As the neutron star encounters the high-density region surrounding the helium core of its massive companion, the rate of energy loss from the orbit increases dramatically leading to either partial or nearly total envelope ejection. The outcome of the common envelope phase depends upon the structure of the evolved companion. In particular, it is found that the entire common envelope can be ejected by the interaction of the neutron star with a red supergiant companion in binaries with orbital periods similar to those of long-period Be X-ray binaries. For orbital periods greater than or approximately equal to 0.8-2 yr (for companions of mass 12-24 solar mass) it is likely that a binary will survive the common envelope phase. For these systems, the structure of the progenitor star is characterized by a steep density gradient above the helium core, and the common envelope phase ends with a spin up of the envelope to within 50%-60% of corotation and with a slow mass outflow. The efficiency of mass ejection is found to be approximately 30%-40%. For less evolved companions, there is insufficient energy in the orbit to unbind the common envelope and only a fraction of it is ejected. Since the timescale for orbital decay is always shorter than the mass-loss timescale from the common envelope, the two cores will likely merge to form a Thorne-Zytkow object. Implications for the origin of Cyg X-3, an X-ray source consisting of a Wolf-Rayet star and a compact companion, and for the fate of the remnant binary consisting of a helium star and a neutron star are briefly discussed.

Resonant Tidal Forcing in Close Binaries: Implications for CVs

NASA Astrophysics Data System (ADS)

Ford, K. E. Saavik; McKernan, Barry; Schwab, Elliana

2018-01-01

Resonant tidal forcing occurs when the tidal forcing frequency of a binary matches a quadrupolar oscillation mode of one of the binary members and energy is transferred from the orbit of the binary to the mode. Tidal locking permits ongoing resonant driving of modes even as binary orbital parameters change. At small binary separations during tidal lock, a significant fraction of binary orbital energy can be deposited quickly into a resonant mode and the binary decays faster than via the emission of gravitational radiation alone. Here we discuss some of the implications of resonant tidal forcing for the class of binaries known as Cataclysmic Variable (CV) stars. We show that resonant tidal forcing of the donor’s Roche lobe could explain the observed 2‑3hr period gap in CVs, assuming modest orbital eccentricities are allowed (eb ∼ 0.03), and can be complementary or an alternative to, existing models. Sudden collapse of the companion orbit, yielding a Type Ia supernova is disfavoured, since Hydrogen is not observed in Type Ia supernova spectra. Therefore, resonance must generally be truncated, probably via mass loss from the Roche lobe or orbital perturbation, ultimately producing a short period CV containing an ’overheated’ white dwarf.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pritychenko, B.

The precision of double-beta ββ-decay experimental half lives and their uncertainties is reanalyzed. The method of Benford's distributions has been applied to nuclear reaction, structure and decay data sets. First-digit distribution trend for ββ-decay T 2v 1/2 is consistent with large nuclear reaction and structure data sets and provides validation of experimental half-lives. A complementary analysis of the decay uncertainties indicates deficiencies due to small size of statistical samples, and incomplete collection of experimental information. Further experimental and theoretical efforts would lead toward more precise values of-decay half-lives and nuclear matrix elements.

General simulation algorithm for autocorrelated binary processes.

PubMed

Serinaldi, Francesco; Lombardo, Federico

2017-02-01

The apparent ubiquity of binary random processes in physics and many other fields has attracted considerable attention from the modeling community. However, generation of binary sequences with prescribed autocorrelation is a challenging task owing to the discrete nature of the marginal distributions, which makes the application of classical spectral techniques problematic. We show that such methods can effectively be used if we focus on the parent continuous process of beta distributed transition probabilities rather than on the target binary process. This change of paradigm results in a simulation procedure effectively embedding a spectrum-based iterative amplitude-adjusted Fourier transform method devised for continuous processes. The proposed algorithm is fully general, requires minimal assumptions, and can easily simulate binary signals with power-law and exponentially decaying autocorrelation functions corresponding, for instance, to Hurst-Kolmogorov and Markov processes. An application to rainfall intermittency shows that the proposed algorithm can also simulate surrogate data preserving the empirical autocorrelation.

Confirmation of the Decay of 283112 and First Indication for Hg-like Behavior of Element 112

NASA Astrophysics Data System (ADS)

Eichler, R.; Aksenov, N. V.; Belozerov, A. V.; Bozhikov, G. A.; Chepigin, V. I.; Dressler, R.; Dmitriev, S. N.; Gäggeler, H. W.; Gorshkov, V. A.; Haenssler, F.; Itkis, M. G.; Lebedev, V. Ya.; Laube, A.; Malyshev, O. N.; Oganessian, Yu. Ts.; Petruschkin, O. V.; Piguet, D.; Rasmussen, P.; Shishkin, S. V.; Shutov, A. V.; Svirikhin, A. I.; Tereshatov, E. E.; Vostokin, G. K.; Wegrzecki, M.; Yeremin, A. V.

2007-05-01

Two gas phase adsorption chemistry experiments aimed at the chemical characterization of element 112 using its isotope 283112 have been performed at the Flerov Laboratory for Nuclear Reactions (FLNR) Dubna, Russia. The applied Insitu-Volatilization and On-line Detection (IVO) technique is a thermochromatographic system combining the determination of the deposition temperature of volatile elements on a surface along a temperature gradient with an efficient detection of the deposited species by event-by-event alpha and SF-fragment spectroscopy. Two possibilities to produce the isotope 283112 were used: 1.) the direct production reaction 238U( 48Ca,3n) 283112; 2.) the reaction 242Pu( 48Ca,3n), where the primary product 287114, decays via alpha emission to 283112 with a half-life of 0.5 s. The chemistry experiments were aimed at a chemical identification of 283112 and an independent confirmation of its decay properties. In the direct reaction no decays related to 283112 were observed. However, two decay chains unambiguously attributed to the decay of 283112 were observed using the second production path. Previously reported observation of 283112 and 279Ds and their decay properties were confirmed. From its thermochromatorgaphic deposition first thermochemical data were deduced for element 112, unveiling it as a typical group 12 element.

Levels in 223Th populated by α decay of 227U

NASA Astrophysics Data System (ADS)

Kalaninová, Z.; Antalic, S.; Heßberger, F. P.; Ackermann, D.; Andel, B.; Kindler, B.; Laatiaoui, M.; Lommel, B.; Maurer, J.

2015-07-01

Levels in 223Th populated by the α decay of 227U were investigated using α -γ decay spectroscopy. The 227U isotope was produced in the fusion-evaporation reaction 22Ne +208Pb at the velocity filter separator for heavy-ion reaction products at Gesellschaft für Schwerionenforschung in Darmstadt (Germany). Several new excited levels and γ transitions were identified in 223Th . An improved α -decay scheme of 227U was suggested. The experimental α -decay energy spectrum of 227U was compared with the Monte Carlo simulation performed using the toolkit geant4.

Beta-Decay Rates for Exotic Nuclei and R-Process Nucleosynthesis up to Th and U

NASA Astrophysics Data System (ADS)

Suzuki, Toshio; Yoshida, Takashi; Shibagaki, Shota; Kajino, Toshitaka; Otsuka, Takaharu

Beta-decay rates for exotic nuclei with N = 126 relevant to r-process nucleosynthesis are studied up to Z = 78 by shell-model calculations. The half-lives for the waiting-point nuclei obtained, which are short compared to a standard FRDM, are used to study r-process nucleosynthesis in neutrino-driven winds and magneto-hydrodynamic jets of core-collapse supernova explosions as well as in binary neutron star mergers. The element abundances are obtained up to the third peak as well as beyond the peak region up to thorium and uranium. Thorium and uranium are found to be produced more with the shorter shell-model half-lives and their abundances come closer to the observed values in core-collapse supernova explosions, while in case of binary neutron star mergers they are produced as much as the observed values rather independent of the half-lives.

Materials Outgassing Rate Decay in Vacuum at Isothermal Conditions

NASA Technical Reports Server (NTRS)

Huang, Alvin Y.; Kastanas, George N.; Kramer, Leonard; Soares, Carlos E.; Mikatarian, Ronald R.

2016-01-01

As a laboratory for scientific research, the International Space Station has been in Low Earth Orbit for nearly 20 years and is expected to be on-orbit for another 10 years. The ISS has been maintaining a relatively pristine contamination environment for science payloads. Materials outgassing induced contamination is currently the dominant source for sensitive surfaces on ISS and modeling the outgassing rate decay over a 20 to 30 year period is challenging. Materials outgassing is described herein as a diffusion-reaction process using ASTM E 1559 rate data. The observation of -1/2 (diffusion) or non-integers (reaction limited) as rate decay exponents for common ISS materials indicate classical reaction kinetics is unsatisfactory in modeling materials outgassing. Non-randomness of reactant concentrations at the interface is the source of this deviation from classical reaction kinetics. A diffusion limited decay was adopted as the result of the correlation of the contaminant layer thicknesses on returned ISS hardware, the existence of high outgassing silicone exhibiting near diffusion limited decay, and the confirmation of non-depleted material after ten years in the Low Earth Orbit.Keywords: Materials Outgassing, ASTM E 1559, Reaction Kinetics, Diffusion, Space Environments Effects, Contamination

Development of a Monte Carlo code for the data analysis of the {sup 18}F(p,α){sup 15}O reaction at astrophysical energies

DOE Office of Scientific and Technical Information (OSTI.GOV)

Caruso, A.; Cherubini, S.; Spitaleri, C.

Novae are astrophysical events (violent explosion) occurring in close binary systems consisting of a white dwarf and a main-sequence star or a star in a more advanced stage of evolution. They are called 'narrow systems' because the two components interact with each other: there is a process of mass exchange with resulting in the transfer of matter from the companion star to the white dwarf, leading to the formation of this last of the so-called accretion disk, rich mainly of hydrogen. Over time, more and more material accumulates until the pressure and the temperature reached are sufficient to trigger nuclearmore » fusion reactions, rapidly converting a large part of the hydrogen into heavier elements. The products of 'hot hydrogen burning' are then placed in the interstellar medium as a result of violent explosions. Studies on the element abundances observed in these events can provide important information about the stages of evolution stellar. During the outbursts of novae some radioactive isotopes are synthesized: in particular, the decay of short-lived nuclei such as {sup 13}N and {sup 18}F with subsequent emission of gamma radiation energy below 511 keV. The gamma rays from products electron-positron annihilation of positrons emitted in the decay of {sup 18}F are the most abundant and the first observable as soon as the atmosphere of the nova starts to become transparent to gamma radiation. Hence the importance of the study of nuclear reactions that lead both to the formation and to the destruction of {sup 18}F. Among these, the {sup 18}F(p,α){sup 15}O reaction is one of the main channels of destruction. This reaction was then studied at energies of astrophysical interest. The experiment done at Riken, Japan, has as its objective the study of the {sup 18}F(p,α){sup 15}O reaction, using a beam of {sup 18}F produced at CRIB, to derive important information about the phenomenon of novae. In this paper we present the experimental technique and the Monte Carlo code developed to be used in the data analysis process.« less

Arrhenius' law in turbulent media and an equivalent tunnel effect. [in binary exchange chemical reactions

NASA Technical Reports Server (NTRS)

Tsuge, S.; Sagara, K.

1978-01-01

The indeterminacy inherent to the formal extension of Arrhenius' law to reactions in turbulent flows is shown to be surmountable in the case of a binary exchange reaction with a sufficiently high activation energy. A preliminary calculation predicts that the turbulent reaction rate is invariant in the Arrhenius form except for an equivalently lowered activation energy. This is a reflection of turbulence-augmented molecular vigor, and causes an appreciable increase in the reaction rate. A similarity to the tunnel effect in quantum mechanics is indicated. The anomaly associated with the mild ignition of oxy-hydrogen mixtures is discussed in this light.

Partial Accretion in the Propeller Stage of Low-mass X-Ray Binary Aql X–1

DOE Office of Scientific and Technical Information (OSTI.GOV)

Güngör, C.; Ekşi, K. Y.; Göğüş, E.

Aql X–1 is one of the most prolific low-mass X-ray binary transients (LMXBTs) showing outbursts almost annually. We present the results of our spectral analyses of Rossi X-Ray Timing Explorer /proportional counter-array observations of the 2000 and 2011 outbursts. We investigate the spectral changes related to the changing disk-magnetosphere interaction modes of Aql X–1. The X-ray light curves of the outbursts of LMXBTs typically show phases of fast rise and exponential decay. The decay phase shows a “knee” where the flux goes from the slow-decay to the rapid-decay stage. We assume that the rapid decay corresponds to a weak propellermore » stage at which a fraction of the inflowing matter in the disk accretes onto the star. We introduce a novel method for inferring, from the light curve, the fraction of the inflowing matter in the disk that accretes onto the neutron star depending on the fastness parameter. We determine the fastness parameter range within which the transition from the accretion to the partial propeller stage is realized. This fastness parameter range is a measure of the scale height of the disk in units of the inner disk radius. We applied the method to a sample of outbursts of Aql X–1 with different maximum flux and duration times. We show that different outbursts with different maximum luminosity and duration follow a similar path in the parameter space of accreted/inflowing mass flux fraction versus fastness parameter.« less

Solvent Dependent Dynamics of Salicylidene Aniline in Binary Mixtures of Supercritical CO2 with 1-Propanol or Cyclohexane.

PubMed

Kieda, Ryan D; Dunkelberger, Adam D; Case, Amanda S; Crim, F Fleming

2017-02-02

The role of different solvent environments in determining the behavior of molecules in solution is a fundamental aspect of chemical reactivity. We present an approach for exploring the influence of solvent properties on condensed-phase dynamics using ultrafast transient absorption spectroscopy in supercritical CO 2 . Using supercritical CO 2 permits adjustment of the density, by varying the temperature and pressure, whereas varying the concentration or identity of a second solvent, the cosolvent, in a binary mixture allows for adjustments of the degree of interaction between the solute and the solvent. Salicylidene aniline, a prototypical excited-state intramolecular proton-transfer system, is the subject of this study. In this system, the decay rate of the transient absorption signal decreases as the fraction of the cosolvent (for both 1-propanol and cyclohexane) increases. The decay rate also decreases with an increase in the viscosity of the mixture, but the effect is much larger for the 1-propanol cosolvent than for cyclohexane. These observations illustrate that the decay rate of the photoexcited salicylidene aniline depends on more than just the solvent viscosity, suggesting that properties such as polarity also play a role in the dynamics.

Towards constructing multi-bit binary adder based on Belousov-Zhabotinsky reaction

NASA Astrophysics Data System (ADS)

Zhang, Guo-Mao; Wong, Ieong; Chou, Meng-Ta; Zhao, Xin

2012-04-01

It has been proposed that the spatial excitable media can perform a wide range of computational operations, from image processing, to path planning, to logical and arithmetic computations. The realizations in the field of chemical logical and arithmetic computations are mainly concerned with single simple logical functions in experiments. In this study, based on Belousov-Zhabotinsky reaction, we performed simulations toward the realization of a more complex operation, the binary adder. Combining with some of the existing functional structures that have been verified experimentally, we designed a planar geometrical binary adder chemical device. Through numerical simulations, we first demonstrated that the device can implement the function of a single-bit full binary adder. Then we show that the binary adder units can be further extended in plane, and coupled together to realize a two-bit, or even multi-bit binary adder. The realization of chemical adders can guide the constructions of other sophisticated arithmetic functions, ultimately leading to the implementation of chemical computer and other intelligent systems.

X-Ray Pulsar Studies With RXTE

NASA Technical Reports Server (NTRS)

Rappaport, Saul

2004-01-01

Our activities here at MIT have largely concentrated on four different binary X-ray pulsars: LMC X-4; 4UO352+3O/XPer; 4U0115+63; and X1908+075. We have also recently initiated a search for millisecond X-ray pulsations in RXTE archival data for several bright LMXBs using a new technique. Since this study is just getting under way, we will not report any results here. Using RXTE timing observations of LMC X-4 we have definitively measured, for the first time, the orbital decay of this high-mass X-ray binary. The e-folding decay time scale is very close to lo6 years, comparable to, but somewhat longer than, the corresponding orbital decay times for SMC X-1 and Cen X-3. We find that the orbital decay in LMC X-4 is likely driven by tidal interactions, where the asynchronism between the orbital motion and the rotation of the companion star is maintained by the evolutionary expansion of the companion. Under NASA grant NAGS7479 we carried out RXTE observations of X Per/4U0352+30 in order to track the pulse phase over a one year interval. This effort was successful in tentatively identifying a N 250-day orbital period. However, due to the fact that the observing interval was only somewhat longer than the orbital period, we asked for the observations of X Per to continue as public, or non-proprietary observations. Dr. Jean Swank kindly agreed to the continuation of the observations and they were carried out on a less frequent basis over the next year and a half. After 72 separate observations of X Per, we have the orbital period and semimajor axis firmly determined. In addition, we were able to measure the orbital eccentricity-which turns out to be remarkably small (e = 0.10) for such a wide binary orbit. This has led us establish the birth of a neutron star with a very small (or zero) natal kick.

Measurements of 2νββ decay-matrix elements for mass A=64,76 and A=96 through charge-exchange reactions

NASA Astrophysics Data System (ADS)

Grewe, E.-W.; Frekers, D.

2006-07-01

We have used the (d,He2) charge-exchange reaction to obtain GT +-strength distributions in the nuclei 64Cu, 76As and 96Nb. These nuclei are the intermediate nuclei in the second-order perturbative description of the 64Zn double-beta plus ( β+β+) and the 76Ge and 96Zr double-beta minus ( β-β-) decays. By means of charge-exchange reactions on parent and daughter nucleus the double-beta decay matrix element can be deduced. In this contribution the measured excitation energy spectra are presented.

Exploiting Photo-induced Reactions in Polymer Blends to Create Hierarchically Ordered, Defect-free Materials

ScienceCinema

Balazs, Anna [University of Pittsburgh, Pittsburgh, Pennsylvania, United States

2017-12-09

Computer simulations reveal how photo-induced chemical reactions can be exploited to create long-range order in binary and ternary polymeric materials. The process is initiated by shining a spatially uniform light over a photosensitive AB binary blend, which undergoes both a reversible chemical reaction and phase separation. We then introduce a well-collimated, higher-intensity light source. Rastering this secondary light over the sample locally increases the reaction rate and causes formation of defect-free, spatially periodic structures. These binary structures resemble either the lamellar or hexagonal phases of microphase-separated di-block copolymers. We measure the regularity of the ordered structures as a function of the relative reaction rates for different values of the rastering speed and determine the optimal conditions for creating defect-free structures in the binary systems. We then add a non-reactive homo-polymer C, which is immiscible with both A and B. We show that this component migrates to regions that are illuminated by the secondary, higher-intensity light, allowing us to effectively write a pattern of C onto the AB film. Rastering over the ternary blend with this collimated light now leads to hierarchically ordered patterns of A, B, and C. The findings point to a facile, non-intrusive process for manufacturing high-quality polymeric devices in a low-cost, efficient manner.

On The Validity of the Assumed PDF Method for Modeling Binary Mixing/Reaction of Evaporated Vapor in GAS/Liquid-Droplet Turbulent Shear Flow

NASA Technical Reports Server (NTRS)

Miller, R. S.; Bellan, J.

1997-01-01

An Investigation of the statistical description of binary mixing and/or reaction between a carrier gas and an evaporated vapor species in two-phase gas-liquid turbulent flows is perfomed through both theroetical analysis and comparisons with results from direct numerical simulations (DNS) of a two-phase mixing layer.

National Nuclear Data Center

Science.gov Websites

reaction data Sigma Retrieval & Plotting Nuclear structure & decay Data Nuclear Science References Experimental Unevaluated Nuclear Data List Evaluated Nuclear Structure Data File NNDC databases Ground and isomeric states properties Nuclear structure & decay data journal Nuclear reaction model code Tools and

Dynamical Cluster-decay Model (DCM) applied to 9Li+208Pb reaction

NASA Astrophysics Data System (ADS)

Kaur, Arshdeep; Hemdeep; Kaushal, Pooja; Behera, Bivash R.; Gupta, Raj K.

2017-10-01

The decay mechanism of 217At* formed in 9Li+208Pb reaction is studied within the dynamical cluster-decay model (DCM) at various center-of-mass energies. The aim is to see the behavior of a light neutron-rich radioactive beam on a doubly-magic target nucleus for the (total) fusion cross section σfus and the individual decay channel cross sections. Experimentally, only the isotopic yield of heavy mass residues * 211- 214At [equivalently, the light-particles (LPs) evaporation residue cross sections σxn for x = 3- 6 neutrons emission] are measured, with the fusion-fission (ff) component σff taken zero. For a fixed neck-length parameter ΔR, the only parameter in the DCM, we are able to fit σfus =∑x=16σxn almost exactly for 9Li on 208Pb at all E c . m .'s. However, the observed individual decay channels (3n-6n) are very poorly fitted, with unobserved channels (1n, 2n) and σff strongly over-estimated. Different ΔR values, meaning thereby different reaction time scales, are required to fit individually both the observed and unobserved evaporation residue channels (1n-6n) and σff, but then the compound nucleus (CN) contribution σCN is very small (< 1%), and the non-compound nucleus (nCN) decay cross section σnCN contributes the most towards total σfus (=σCN +σnCN). Thus, the 9Li induced reaction on doubly-magic 208Pb is more of a quasi-fission-like nCN decay, which is further analyzed in terms of the statistical CN formation probability PCN and CN survival probability Psurv. For the reaction under study, PCN < < 1 and Psurv → 1, in particular at above barrier energies.

Modeling CO2 mass transfer in amine mixtures: PZ-AMP and PZ-MDEA.

PubMed

Puxty, Graeme; Rowland, Robert

2011-03-15

The most common method of carbon dioxide (CO(2)) capture is the absorption of CO(2) into a falling thin film of an aqueous amine solution. Modeling of mass transfer during CO(2) absorption is an important way to gain insight and understanding about the underlying processes that are occurring. In this work a new software tool has been used to model CO(2) absorption into aqueous piperazine (PZ) and binary mixtures of PZ with 2-amino-2-methyl-1-propanol (AMP) or methyldiethanolamine (MDEA). The tool solves partial differential and simultaneous equations describing diffusion and chemical reaction automatically derived from reactions written using chemical notation. It has been demonstrated that by using reactions that are chemically plausible the mass transfer in binary mixtures can be fully described by combining the chemical reactions and their associated parameters determined for single amines. The observed enhanced mass transfer in binary mixtures can be explained through chemical interactions occurring in the mixture without need to resort to using additional reactions or unusual transport phenomena such as the "shuttle mechanism".

One-step argon/nitrogen binary plasma jet irradiation of Li4Ti5O12 for stable high-rate lithium ion battery anodes

NASA Astrophysics Data System (ADS)

Lan, Chun-Kai; Chuang, Shang-I.; Bao, Qi; Liao, Yen-Ting; Duh, Jenq-Gong

2015-02-01

Atmospheric pressure Ar/N2 binary plasma jet irradiation has been introduced into the manufacturing process of lithium ions batteries as a facile, green and scalable post-fabrication treatment approach, which enhanced significantly the high-rate anode performance of lithium titanate (Li4Ti5O12). Main emission lines in Ar/N2 plasma measured by optical emission spectroscopy reveal that the dominant excited high-energy species in Ar/N2 plasma are N2*, N2+, N∗ and Ar∗. Sufficient oxygen vacancies have been evidenced by high resolution X-ray photoelectron spectroscopy analysis and Raman spectra. Nitrogen doping has been achieved simultaneously by the surface reaction between pristine Li4Ti5O12 particles and chemically reactive plasma species such as N∗ and N2+. The variety of Li4Ti5O12 particles on the surface of electrodes after different plasma processing time has been examined by grazing incident X-Ray diffraction. Electrochemical impedance spectra (EIS) confirm that the Ar/N2 atmospheric plasma treatment facilitates Li+ ions diffusion and reduces the internal charge-transfer resistance. The as-prepared Li4Ti5O12 anodes exhibit a superior capacity (132 mAh g-1) and excellent stability with almost no capacity decay over 100 cycles under a high C rate (10C).

Refining Binary Pulsar B1913+16's Gravitational Wave Test via a VLBI Parallax Measurement

NASA Astrophysics Data System (ADS)

Weisberg, Joel; Deller, Adam; Chatterjee, Shami; Nice, David

2018-01-01

The orbital decay of binary pulsar B1913+16 provided the first evidence of gravitational waves as predicted by General Relativity, and ruled out numerous previously viable alternative gravitational theories (e.g., Taylor & Weisberg, APJ, 253, 908, 1982). The gravitational wave emission and resulting orbital decay manifest themselves as an orbital period derivative. Subsequent observations (e.g., Weisberg and Huang 2016, APJ, 829, 55) have greatly refined the precision of the orbital period derivative measurement. The accuracy of the experiment is currently limited by our knowledge of the relative galactic accelerations of the binary and solar system barycenters, which make another contribution to the observed orbital period derivative. The magnitude of these accelerations depend on various galactic constants and on the pulsar distance.As our knowledge of the Galaxy and its motions has improved, the pulsar's distance has become the largest remaining source of uncertainty in the experiment.Therefore, we conducted a series of astrometric measurements of PSR B1913+16 with the Very Long Baseline Array. We report the pulsar parallax and distance derived from these measurements, and use them to correct our observed orbital period derivative for the above galactic acceleration term, thereby providing a more accurate test of gravitational radiation emission from the system.

ThermoData Engine Database - Pure Compounds and Binary Mixtures

National Institute of Standards and Technology Data Gateway

SRD 103b NIST ThermoData Engine Version 6.0 - Pure CompoThermoData Engine Database - Pure Compounds and Binary Mixtures (PC database for purchase)   This database contains property data for more than 21,000 pure compounds, 37,500 binary mixtures, 10,000 ternary mixtures, and 6,000 chemical reactions.

The formation of Kuiper-belt binaries through exchange reactions.

PubMed

Funato, Yoko; Makino, Junichiro; Hut, Piet; Kokubo, Eiichiro; Kinoshita, Daisuke

2004-02-05

Recent observations have revealed that an unexpectedly high fraction--a few per cent--of the trans-Neptunian objects (TNOs) that inhabit the Kuiper belt are binaries. The components have roughly equal masses, with very eccentric orbits that are wider than a hundred times the radius of the primary. Standard theories of binary asteroid formation tend to produce close binaries with circular orbits, so two models have been proposed to explain the unique characteristics of the TNOs. Both models, however, require extreme assumptions regarding the size distribution of the TNOs. Here we report a mechanism that is capable of producing binary TNOs with the observed properties during the early stages of their formation and growth. The only required assumption is that the TNOs were initially formed through gravitational instabilities in the protoplanetary dust disk. The basis of the mechanism is an exchange reaction in which a binary whose primary component is much more massive than the secondary interacts with a third body, whose mass is comparable to that of the primary. The low-mass secondary component is ejected and replaced by the third body in a wide but eccentric orbit.

Preparation and application of nanoglued binary titania-silica aerogel.

PubMed

Luo, Liang; Cooper, Adrienne T; Fan, Maohong

2009-01-15

Nanoglued binary titania (TiO2)-silica (SiO2) aerogel, as a novel type of photocatalyst, has been synthesized on glass substrates. Using an about-to-gel SiO2 sol as nanoglue, anatase TiO2 aerogel was immobilized into a three-dimensional mesoporous network of the SiO2. Factorial designs were employed to optimize both TiO2 aerogel and binary TiO2-SiO2 aerogel synthesis. Characterization of the as-prepared TiO2 and binary samples by surface area, porosity, and surface chemical composition showed that the photocatalysts were high-surface-area nanoporous materials, with a Ti4+ valency. The binary aerogel exhibited high photocatalytic activity for the degradation of methylene blue (MB) under simulated solar light; the reaction followed the pseudo first-order Langmuir-Hinshelwood (L-H) kinetic model. Fluorescence spectroscopy revealed that the hydroxyl (*OH) radical was formed during the illumination of the binary TiO2-SiO2 aerogel in a solution of probe molecules, which corroborates the probable mechanism of hydroxyl radical oxidation of contaminants in photocatalytic reactions.

Modification of a method-of-characteristics solute-transport model to incorporate decay and equilibrium-controlled sorption or ion exchange

USGS Publications Warehouse

Goode, D.J.; Konikow, Leonard F.

1989-01-01

The U.S. Geological Survey computer model of two-dimensional solute transport and dispersion in ground water (Konikow and Bredehoeft, 1978) has been modified to incorporate the following types of chemical reactions: (1) first-order irreversible rate-reaction, such as radioactive decay; (2) reversible equilibrium-controlled sorption with linear, Freundlich, or Langmuir isotherms; and (3) reversible equilibrium-controlled ion exchange for monovalent or divalent ions. Numerical procedures are developed to incorporate these processes in the general solution scheme that uses method-of- characteristics with particle tracking for advection and finite-difference methods for dispersion. The first type of reaction is accounted for by an exponential decay term applied directly to the particle concentration. The second and third types of reactions are incorporated through a retardation factor, which is a function of concentration for nonlinear cases. The model is evaluated and verified by comparison with analytical solutions for linear sorption and decay, and by comparison with other numerical solutions for nonlinear sorption and ion exchange.

Materials outgassing rate decay in vacuum at isothermal conditions

NASA Astrophysics Data System (ADS)

Huang, Alvin Y.; Kastanas, George N.; Kramer, Leonard; Soares, Carlos E.; Mikatarian, Ronald R.

2016-09-01

As a laboratory for scientific research, the International Space Station has been in Low Earth Orbit for over 17 years and is planned to be on-orbit for another 10 years. The ISS has been maintaining a relatively pristine contamination environment for science payloads. Materials outgassing induced contamination is currently the dominant source for sensitive surfaces on ISS and modelling the outgassing rate decay over a 20 to 30 year period is challenging. Using ASTM E 1559 rate data, materials outgassing is described herein as a diffusion-reaction process with the interface playing a key role. The observation of -1/2 (diffusion) or non-integers (reaction limited) as rate decay exponents for common ISS materials indicate classical reaction kinetics is unsatisfactory in modelling materials outgassing. Nonrandomness of reactant concentrations at the interface is the source of this deviation from classical reaction kinetics. A t-1/2 decay is adopted as the result of the correlation of the contaminant layer thicknesses and composition on returned ISS hardware, the existence of high outgassing silicone exhibiting near diffusion limited decay, the confirmation of nondepleted material after ten years in Low Earth Orbit, and a potential slowdown of long term materials outgassing kinetics due to silicone contaminants at the interface.

The decay of hot nuclei formed in La-induced reactions at E/A=45 MeV

DOE Office of Scientific and Technical Information (OSTI.GOV)

Libby, Bruce

1993-01-01

The decay of hot nuclei formed in the reactions 139La + 27Al, 51V, natCu, and 139La were studied by the coincident detection of up to four complex fragments (Z > 3) emitted in these reactions. Fragments were characterized as to their atomic number, energy and in- and out-of-plane angles. The probability of the decay by an event of a given complex fragment multiplicity as a function of excitation energy per nucleon of the source is nearly independent of the system studied. Additionally, there is no large increase in the proportion of multiple fragment events as the excitation energy of themore » source increases past 5 MeV/nucleon. This is at odds with many prompt multifragmentation models of nuclear decay. The reactions 139La + 27Al, 51V, natCu were also studied by combining a dynamical model calculation that simulates the early stages of nuclear reactions with a statistical model calculation for the latter stages of the reactions. For the reaction 139La + 27Al, these calculations reproduced many of the experimental features, but other features were not reproduced. For the reaction 139La + 51V, the calculation failed to reproduce somewhat more of the experimental features. The calculation failed to reproduce any of the experimental features of the reaction 139La + natCu, with the exception of the source velocity distributions.« less

The decay of hot nuclei formed in La-induced reactions at E/A=45 MeV

DOE Office of Scientific and Technical Information (OSTI.GOV)

Libby, B.

1993-01-01

The decay of hot nuclei formed in the reactions [sup 139]La + [sup 27]Al, [sup 51]V, [sup nat]Cu, and [sup 139]La were studied by the coincident detection of up to four complex fragments (Z > 3) emitted in these reactions. Fragments were characterized as to their atomic number, energy and in- and out-of-plane angles. The probability of the decay by an event of a given complex fragment multiplicity as a function of excitation energy per nucleon of the source is nearly independent of the system studied. Additionally, there is no large increase in the proportion of multiple fragment events asmore » the excitation energy of the source increases past 5 MeV/nucleon. This is at odds with many prompt multifragmentation models of nuclear decay. The reactions [sup 139]La + [sup 27]Al, [sup 51]V, [sup nat]Cu were also studied by combining a dynamical model calculation that simulates the early stages of nuclear reactions with a statistical model calculation for the latter stages of the reactions. For the reaction [sup 139]La + [sup 27]Al, these calculations reproduced many of the experimental features, but other features were not reproduced. For the reaction [sup 139]La + [sup 51]V, the calculation failed to reproduce somewhat more of the experimental features. The calculation failed to reproduce any of the experimental features of the reaction [sup 139]La + [sup nat]Cu, with the exception of the source velocity distributions.« less

Enzymatic synthesis of 6-O-glucosyl-poly(3-hydroxyalkanoate) in organic solvents and their binary mixture.

PubMed

Gumel, A M; Annuar, M S M; Heidelberg, T

2013-04-01

The effects of organic solvents and their binary mixture in the glucose functionalization of bacterial poly-3-hydroxyalkanoates catalyzed by Lecitase™ Ultra were studied. Equal volume binary mixture of DMSO and chloroform with moderate polarity was more effective for the enzyme catalyzed synthesis of the carbohydrate polymer at ≈38.2 (±0.8)% reactant conversion as compared to the mono-phasic and other binary solvents studied. The apparent reaction rate constant as a function of medium water activity (aw) was observed to increase with increasing solvent polarity, with optimum aw of 0.2, 0.4 and 0.7 (±0.1) observed in hydrophilic DMSO, binary mixture DMSO:isooctane and hydrophobic isooctane, respectively. Molecular sieve loading between 13 to 15gL(-1) (±0.2) and reaction temperature between 40 to 50°C were found optimal. Functionalized PHA polymer showed potential characteristics and biodegradability. Copyright © 2012 Elsevier B.V. All rights reserved.

β-decay Rates for Exotic Nuclei and r-process Nucleosynthesis up to Thorium and Uranium

NASA Astrophysics Data System (ADS)

Suzuki, Toshio; Shibagaki, Shota; Yoshida, Takashi; Kajino, Toshitaka; Otsuka, Takaharu

2018-06-01

Beta-decay rates for exotic nuclei with neutron magic number of N = 126 relevant to r-process nucleosynthesis are studied up to Z = 78 by shell-model calculations. The half-lives for the waiting-point nuclei obtained, which are short compared to a standard finite-range-droplet model, are used to study r-process nucleosynthesis in core-collapse supernova (CCSN) explosions and binary neutron star mergers. The element abundances are obtained up to the third peak as well as beyond the peak region up to thorium and uranium. The position of the third peak is found to be shifted toward a higher mass region in both CCSN explosions and neutron star mergers. We find that thorium and uranium elements are produced more with the shorter shell-model half-lives and their abundances come close to the observed values in CCSN explosions. In the case of binary neutron star mergers, thorium and uranium are produced consistently with the observed values independent of the half-lives.

A possible macronova in the late afterglow of the long-short burst GRB 060614.

PubMed

Yang, Bin; Jin, Zhi-Ping; Li, Xiang; Covino, Stefano; Zheng, Xian-Zhong; Hotokezaka, Kenta; Fan, Yi-Zhong; Piran, Tsvi; Wei, Da-Ming

2015-06-11

Long-duration (>2 s) γ-ray bursts that are believed to originate from the death of massive stars are expected to be accompanied by supernovae. GRB 060614, that lasted 102 s, lacks a supernova-like emission down to very stringent limits and its physical origin is still debated. Here we report the discovery of near-infrared bump that is significantly above the regular decaying afterglow. This red bump is inconsistent with even the weakest known supernova. However, it can arise from a Li-Paczyński macronova--the radioactive decay of debris following a compact binary merger. If this interpretation is correct, GRB 060614 arose from a compact binary merger rather than from the death of a massive star and it was a site of a significant production of heavy r-process elements. The significant ejected mass favours a black hole-neutron star merger but a double neutron star merger cannot be ruled out.

Particle decay of proton-unbound levels in N 12

DOE PAGES

Chipps, K. A.; Pain, S. D.; Greife, U.; ...

2017-04-24

Transfer reactions are a useful tool for studying nuclear structure, particularly in the regime of low level densities and strong single-particle strengths. Additionally, transfer reactions can populate levels above particle decay thresholds, allowing for the possibility of studying the subsequent decays and furthering our understanding of the nuclei being probed. In particular, the decay of loosely bound nuclei such as 12 N can help inform and improve structure models.The purpose of this paper is to learn about the decay of excited states in 12 N , to more generally inform nuclear structure models, particularly in the case of particle-unbound levelsmore » in low-mass systems which are within the reach of state-of-the-art ab initio calculations.« less

A note on implementation of decaying product correlation structures for quasi-least squares.

PubMed

Shults, Justine; Guerra, Matthew W

2014-08-30

This note implements an unstructured decaying product matrix via the quasi-least squares approach for estimation of the correlation parameters in the framework of generalized estimating equations. The structure we consider is fairly general without requiring the large number of parameters that are involved in a fully unstructured matrix. It is straightforward to show that the quasi-least squares estimators of the correlation parameters yield feasible values for the unstructured decaying product structure. Furthermore, subject to conditions that are easily checked, the quasi-least squares estimators are valid for longitudinal Bernoulli data. We demonstrate implementation of the structure in a longitudinal clinical trial with both a continuous and binary outcome variable. Copyright © 2014 John Wiley & Sons, Ltd.

Radical Abstraction Reactions with Concerted Fragmentation in the Chain Decay of Nitroalkanes

NASA Astrophysics Data System (ADS)

Denisov, E. T.; Shestakov, A. F.

2018-05-01

Reactions of the type X• + HCR2CH2NO2 → XH + R2C=CH2 + N•O2 are exothermic, due to the breaking of weak C-N bonds and the formation of energy-intensive C=C bonds. Quantum chemistry calculations of the transition state using the reactions of Et• and EtO• with 2-nitrobutane shows that such reactions can be categorized as one-step, due to the extreme instability of the intermediate nitrobutyl radical toward decay with the formation of N•O2. Kinetic parameters that allow us to calculate the energy of activation and rate constant of such a reaction from its enthalpy are estimated using a model of intersecting parabolas. Enthalpies, energies of activation, and rate constants are calculated for a series of reactions with the participation of Et•, EtO•, RO•2, N•O2 radicals on the one hand and a series of nitroalkanes on the other. A new kinetic scheme of the chain decay of nitroalkanes with the participation of abstraction reactions with concerted fragmentation is proposed on the basis of the obtained data.

Simple method for quantifying microbiologically assisted chloramine decay in drinking water.

PubMed

Sathasivan, Arumugam; Fisher, Ian; Kastl, George

2005-07-15

In a chloraminated drinking water distribution system, monochloramine decays due to chemical and microbiological reactions. For modeling and operational control purposes, it is necessary to know the relative contribution of each type of reaction, but there was no method to quantify these contributions separately. A simple method was developed to do so. It compares monochloramine decay rates of processed (0.2 microm filtered or microbiologically inhibited by adding 100 microg of silver/L as silver nitrate) and unprocessed samples under controlled temperature conditions. The term microbial decay factor (Fm) was defined and derived from this method, to characterize the relative contribution of microbiologically assisted monochloramine decay to the total monochloramine decay observed in bulk water. Fm is the ratio between microbiologically assisted monochloramine decay and chemical decay of a given water sample measured at 20 degrees C. One possible use of the method is illustrated, where a service reservoir's bulk and inlet waters were sampled twice and analyzed for both the traditional indicators and the microbial decay factor. The microbial decay factor values alone indicated that more microbiologically assisted monochloramine decay was occurring in one bulk water than the other. In contrast, traditional nitrification indicators failed to show any difference. Further analysis showed that the microbial decay factor is more sensitive and that it alone can provide an early warning.

Observation of the hc(1P1) state of charmonium.

PubMed

Rosner, J L; Adam, N E; Alexander, J P; Berkelman, K; Cassel, D G; Crede, V; Duboscq, J E; Ecklund, K M; Ehrlich, R; Fields, L; Galik, R S; Gibbons, L; Gittelman, B; Gray, R; Gray, S W; Hartill, D L; Heltsley, B K; Hertz, D; Jones, C D; Kandaswamy, J; Kreinick, D L; Kuznetsov, V E; Mahlke-Krüger, H; Meyer, T O; Onyisi, P U E; Patterson, J R; Peterson, D; Phillips, E A; Pivarski, J; Riley, D; Ryd, A; Sadoff, A J; Schwarthoff, H; Shi, X; Shepherd, M R; Stroiney, S; Sun, W M; Urner, D; Wilksen, T; Weaver, K M; Weinberger, M; Athar, S B; Avery, P; Breva-Newell, L; Patel, R; Potlia, V; Stoeck, H; Yelton, J; Rubin, P; Cawlfield, C; Eisenstein, B I; Gollin, G D; Karliner, I; Kim, D; Lowrey, N; Naik, P; Sedlack, C; Selen, M; White, E J; Williams, J; Wiss, J; Edwards, K W; Besson, D; Pedlar, T K; Cronin-Hennessy, D; Gao, K Y; Gong, D T; Hietala, J; Kubota, Y; Klein, T; Lang, B W; Li, S Z; Poling, R; Scott, A W; Smith, A; Dobbs, S; Metreveli, Z; Seth, K K; Tomaradze, A; Zweber, P; Ernst, J; Mahmood, A H; Severini, H; Asner, D M; Dytman, S A; Love, W; Mehrabyan, S; Mueller, J A; Savinov, V; Li, Z; Lopez, A; Mendez, H; Ramirez, J; Huang, G S; Miller, D H; Pavlunin, V; Sanghi, B; Shipsey, I P J; Adams, G S; Cravey, M; Cummings, J P; Danko, I; Napolitano, J; He, Q; Muramatsu, H; Park, C S; Park, W; Thorndike, E H; Coan, T E; Gao, Y S; Liu, F; Artuso, M; Boulahouache, C; Blusk, S; Butt, J; Dorjkhaidav, O; Li, J; Menaa, N; Mountain, R; Nandakumar, R; Randrianarivony, K; Redjimi, R; Sia, R; Skwarnicki, T; Stone, S; Wang, J C; Zhang, K; Csorna, S E; Bonvicini, G; Cinabro, D; Dubrovin, M; Briere, R A; Chen, G P; Chen, J; Ferguson, T; Tatishvili, G; Vogel, H; Watkins, M E

2005-09-02

The h(c)((1)P(1)) state of charmonium has been observed in the reaction psi(2S) --> pi(0)h(c) --> (gammagamma)(gammaeta(c)) using 3.08 x10(6) psi(2S) decays recorded in the CLEO detector. Data have been analyzed both for the inclusive reaction, where the decay products of the eta(c) are not identified, and for exclusive reactions, in which eta(c) decays are reconstructed in seven hadronic decay channels. We find M(h(c)) = 3524.4 +/- 0.6 +/- 0.4 MeV which corresponds to a hyperfine splitting DeltaM(hf)(1P) triple-bond pi(0)h(c)) x B(h(c) --> gammaeta(c)) = (4.0 +/- 0.8 +/- 0.7) x 10(-4).

Probing Neutron Star Evolution with Gamma Rays

NASA Astrophysics Data System (ADS)

Wijers, Ralph A. M. J.

1996-02-01

The research sponsored by this grant was conducted in two fields of high-energy astrophysics: gamma-ray bursts and evolution of neutron stars. It is unknown at this time whether they are related. The work performed in each area is discussed followed by a full list of publications supported by the grant. My research (with E. Fenimore, L. Lubin, B. Paczyiiski, and A. Ulmer) has focussed on devising tests that could distinguish between BATSE and galactic-halo distance scales using the available data. In the first instance, the issue was whether the early BATSE peak flux distribution could be used to extract more than just a slope of the log N(greater than P) distribution, and whether it joined smoothly to the steeper peak flux distribution of bright bursts. To this end, we analysed the peak flux distribution for the presence of a change in slope. This was done both by fitting models with a core radius to see whether a significant value for it could be found, and by developing a completely model-independent test to search for slope changes in arbitrary distributions that are nearly power laws. A slope change was marginally detected in the first-year BATSE data. Good progress has been made in understanding the evolution of neutron stars and their magnetic fields. Having shown in earlier work that magnetic fields in some neutron stars, particularly Her X-1, do not decay spontaneously on million-year time scales, we set out to check whether such spontaneous decay was needed in isolated radio pulsars, as claimed by many. We found that it is not; rather long decay times or no decay are preferred. Since there are neutron stars with low magnetic fields, one must conclude that there is something in their past that distinguishes them from most pulsars. These so-called recycled pulsars are in binaries much more often than normal pulsars. My research concentrates on the class of scenarios in which the recycled pulsars are initially the same as ordinary high-field radio pulsars, and have acquired their properties due to mass transfer processes in binary stars. This links their evolution to that of X-ray binaries.

The 76Ge(n,p)76Ga reaction and its relevance to searches for the neutrino-less double-beta decay of 76Ge

NASA Astrophysics Data System (ADS)

Tornow, W.; Bhike, Megha; Fallin, B.; Krishichayan, Fnu

2015-10-01

The 76Ge(n,p)76Ga reaction and the subsequent β decay of 76Ga to 76Ge has been used to excite the 3951.9 keV state of 76Ge, which decays by emission of a 2040.7 keV γ ray. Using HPGe detectors, the associated pulse-height signal may be undistinguishable from the potential signal produced in neutrino-less double-beta decay of 76Ge with its Q-value of 2039.0 keV. In the neutron energy range between 10 and 20 MeV the production cross section of the 2040.7 keV γ ray is approximately 0.1 mb. In the same experiment γ rays of energy 2037.9 keV resulting from the 76Ge(n, γ)77Ge reaction were clearly observed. Adding the 76Ge(n,n' γ)76Ge reaction, which also produces the 2040.7 keV γ ray with a cross section value of the order of 0.1 mb clearly shows that great care has to be taken to eliminate neutron-induced backgrounds in searches for neutrino-less double-beta decay of 76Ge. This work was supported by the U.S. DOE under Grant NO. DE-FG02-97ER41033.

Modelling Chemical Reasoning to Predict and Invent Reactions.

PubMed

Segler, Marwin H S; Waller, Mark P

2017-05-02

The ability to reason beyond established knowledge allows organic chemists to solve synthetic problems and invent novel transformations. Herein, we propose a model that mimics chemical reasoning, and formalises reaction prediction as finding missing links in a knowledge graph. We have constructed a knowledge graph containing 14.4 million molecules and 8.2 million binary reactions, which represents the bulk of all chemical reactions ever published in the scientific literature. Our model outperforms a rule-based expert system in the reaction prediction task for 180 000 randomly selected binary reactions. The data-driven model generalises even beyond known reaction types, and is thus capable of effectively (re-)discovering novel transformations (even including transition metal-catalysed reactions). Our model enables computers to infer hypotheses about reactivity and reactions by only considering the intrinsic local structure of the graph and because each single reaction prediction is typically achieved in a sub-second time frame, the model can be used as a high-throughput generator of reaction hypotheses for reaction discovery. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

X-Ray Timing Analysis of Cyg X-3 Using AstroSat/LAXPC: Detection of Milli-hertz Quasi-periodic Oscillations during the Flaring Hard X-Ray State

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pahari, Mayukh; Misra, Ranjeev; Antia, H M

We present here results from the X-ray timing and spectral analysis of the X-ray binary Cyg X-3 using observations from the Large Area X-ray proportional Counter on board AstroSat . Consecutive light curves observed over a period of one year show the binary orbital period of 17253.56 ± 0.19 s. Another low-amplitude, slow periodicity of the order of 35.8 ± 1.4 days is observed, which may be due to the orbital precession as suggested earlier by Molteni et al. During the rising binary phase, power density spectra from different observations during the flaring hard X-ray state show quasi-periodic oscillations (QPOs)more » at ∼5–8 mHz, ∼12–14 mHz, and ∼18–24 mHz frequencies at the minimum confidence of 99%. However, during the consecutive binary decay phase, no QPO is detected up to 2 σ significance. Energy-dependent time-lag spectra show soft lag (soft photons lag hard photons) at the mHz QPO frequency and the fractional rms of the QPO increases with the photon energy. During the binary motion, the observation of mHz QPOs during the rising phase of the flaring hard state may be linked to the increase in the supply of the accreting material in the disk and corona via stellar wind from the companion star. During the decay phase, the compact source moves in the outer wind region causing the decrease in supply of material for accretion. This may cause weakening of the mHz QPOs below the detection limit. This is also consistent with the preliminary analysis of the orbital phase-resolved energy spectra presented in this paper.« less

Orbital evolution and search for eccentricity and apsidal motion in the eclipsing HMXB 4U 1700-37

NASA Astrophysics Data System (ADS)

Islam, Nazma; Paul, Biswajit

2016-09-01

In the absence of detectable pulsations in the eclipsing high-mass X-ray binary 4U 1700-37, the orbital period decay is necessarily determined from the eclipse timing measurements. We have used the earlier reported mid-eclipse time measurements of 4U 1700-37 together with the new measurements from long-term light curves obtained with the all sky monitors RXTE-ASM, Swift-BAT and MAXI-GSC, as well as observations with RXTE-PCA, to measure the long-term orbital evolution of the binary. The orbital period decay rate of the system is estimated to be {dot{P}}/P = -(4.7 ± 1.9) × 10^{-7} yr-1, smaller compared to its previous estimates. We have also used the mid-eclipse times and the eclipse duration measurements obtained from 10-years-long X-ray light curve with Swift-BAT to separately put constraints on the eccentricity of the binary system and attempted to measure any apsidal motion. For an apsidal motion rate greater than 5 deg yr-1, the eccentricity is found to be less than 0.008, which limits our ability to determine the apsidal motion rate from the current data. We discuss the discrepancy of the current limit of eccentricity with the earlier reported values from radial velocity measurements of the companion star.

Informing neutron capture nucleosynthesis on short-lived nuclei with (d,p) reactions

NASA Astrophysics Data System (ADS)

Cizewski, Jolie A.; Ratkiewicz, Andrew; Escher, Jutta E.; Lepailleur, Alexandre; Pain, Steven D.; Potel, Gregory

2018-01-01

Neutron capture on unstable nuclei is important in understanding abundances in r-process nucleosynthesis. Previously, the non-elastic breakup of the deuteron in the (d,p) reaction has been shown to provide a neutron that can be captured by the nucleus and the gamma-ray decay of the subsequent compound nucleus can be modelled to predict the gamma-ray decay of the compound nucleus in the (n,γ) reaction. Preliminary results from the 95Mo(d,pγ) reaction in normal kinematics support the (d,pγ) reaction as a valid surrogate for neutron capture. The techniques to measure the (d,pγ) reaction in inverse kinematics have been developed.

Experimental evidence of the 6He level at E*=18.3 MeV via the 4He + 3H three-body reaction

NASA Astrophysics Data System (ADS)

Povoroznyk, O. M.; Gorpinich, O. K.; Jachmenjov, O. O.; Mokhnach, H. V.; Ponkratenko, O.; Mandaglio, G.; Curciarello, F.; De Leo, V.; Fazio, G.; Giardina, G.

2012-06-01

Measurements of the t-t and p-t coincidence events in the 3H (α,tt)1H reaction have been obtained at incident energy Eα=67.2 MeV. Various appropriate angular configurations of detectors were chosen in order to observe the population of the 6He* state at around 18 MeV. Its contribution appears at the relative energy of Ett=6.0 MeV as found from an analysis of the bidimensional spectra. We found the formation of the 6He excited state at E*=18.3±0.2 MeV (with a Γ width of 1.1 ± 0.3 MeV) by using the decay into the t+t binary channel, since the threshold energy of the t+t channel is 12.31 MeV. In each analyzed bidimensional energy spectrum of (Et, Et) and (Ep, Et) coincidence events, resonance structures are present due to the formation of both 6He* and 4He* excited states. Our results on the E* and Γ values regarding the 6He* level of about 18 MeV are compared with the results obtained using other reactions. Moreover, we also found new Γ width values of 0.7 ± 0.3 and 0.8 ± 0.4 MeV for the 14.0 ± 0.4 and 16.1 ± 0.4 MeV 6He levels, respectively.

Configuration interaction calculations for the region of 76Ge

NASA Astrophysics Data System (ADS)

Brown, Alex

2017-09-01

I will present a short history of the configuration interaction Hamiltonians that have been developed for the (0f5 / 2 , 1p3 / 2 , 1p1 / 2 , 0g9 / 2) (jj 44) model space. This model space is appropriate for the region of nuclei bounded by the nickel isotopes for Z = 28 and the isotones with N = 50 . I will discuss results for the double-beta decay of 76Ge that lies in the jj 44 region. I will show results for the structure of nuclei around 76Ge for some selected data from gamma decay, Gamow-Teller beta decay, charge-exchange reactions, one-nucleon transfer reactions, and two-nucleon transfer reactions. This work was supported by NSF Grant PHY-1404442.

Pycnonuclear reaction rates for binary ionic mixtures

NASA Technical Reports Server (NTRS)

Ichimaru, S.; Ogata, S.; Van Horn, H. M.

1992-01-01

Through a combination of compositional scaling arguments and examinations of Monte Carlo simulation results for the interparticle separations in binary-ionic mixture (BIM) solids, we have derived parameterized expressions for the BIM pycnonuclear rates as generalizations of those in one-component solids obtained previously by Salpeter and Van Horn and by Ogata et al. We have thereby discovered a catalyzing effect of the heavier elements, which enhances the rates of reactions among the lighter elements when the charge ratio exceeds a critical value of approximately 2.3.

Late-time X-ray signatures of compact binary mergers: potential counterparts of gravitational wave events

NASA Astrophysics Data System (ADS)

Tanvir, Nial

2017-09-01

Merging compact binaries (NS-NS or NS-BH) offer the best prospects for detection of EM signals accompanying gravitational wave (GW) events. They may be seen as bright short-GRBs (SGRBs), but this is likely to be rare due to beaming. Alternatively, more isotropic near-IR emission is predicted to result from the 'kilonova' produced by radioactive decay of neutron star ejecta. However, recent XMM observations have shown unexplained excess X-ray emission several days post-burst in two low-z SGRBs. This may indicate ongoing engine activity which both enhances the nIR emission, and crucially provides a potential new isotropic X-ray signature of compact binary mergers. We propose a detailed study of a further z<0.35 SGRB, to explore this phenomenon and inform future searches for GW counterparts.

Constraining f(R) gravity in solar system, cosmology and binary pulsar systems

NASA Astrophysics Data System (ADS)

Liu, Tan; Zhang, Xing; Zhao, Wen

2018-02-01

The f (R) gravity can be cast into the form of a scalar-tensor theory, and scalar degree of freedom can be suppressed in high-density regions by the chameleon mechanism. In this article, for the general f (R) gravity, using a scalar-tensor representation with the chameleon mechanism, we calculate the parametrized post-Newtonian parameters γ and β, the effective gravitational constant Geff, and the effective cosmological constant Λeff. In addition, for the general f (R) gravity, we also calculate the rate of orbital period decay of the binary system due to gravitational radiation. Then we apply these results to specific f (R) models (Hu-Sawicki model, Tsujikawa model and Starobinsky model) and derive the constraints on the model parameters by combining the observations in solar system, cosmological scales and the binary systems.

KCTF evolution of trans-neptunian binaries: Connecting formation to observation

NASA Astrophysics Data System (ADS)

Porter, Simon B.; Grundy, William M.

2012-08-01

Recent observational surveys of trans-neptunian binary (TNB) systems have dramatically increased the number of known mutual orbits. Our Kozai Cycle Tidal Friction (KCTF) simulations of synthetic trans-neptunian binaries show that tidal dissipation in these systems can completely reshape their original orbits. Specifically, solar torques should have dramatically accelerated the semimajor axis decay and circularization timescales of primordial (or recently excited) TNBs. As a result, our initially random distribution of TNBs in our simulations evolved to have a large population of tight circular orbits. This tight circular population appears for a range of TNO physical properties, though a strong gravitational quadrupole can prevent some from fully circularizing. We introduce a stability parameter to predict the effectiveness of KCTF on a TNB orbit, and show that a number of known TNBs must have a large gravitational quadrupole to be stable.

β-delayed γ decay of 20Mg and the 19Ne(p , γ) 20 Na breakout reaction in Type I X-ray bursts

NASA Astrophysics Data System (ADS)

Glassman, B. E.; Pérez-Loureiro, D.; Wrede, C.; Allen, J.; Bardayan, D. W.; Bennett, M. B.; Brown, B. A.; Chipps, K. A.; Febbraro, M.; Friedman, M.; Fry, C.; Hall, M. R.; Hall, O.; Liddick, S. N.; O'Malley, P.; Ong, W. J.; Pain, S. D.; Prokop, C.; Schwartz, S. B.; Shidling, P.; Sims, H.; Thompson, P.; Zhang, H.

2018-03-01

Certain astrophysical environments such as thermonuclear outbursts on accreting neutron stars (Type-I X-ray bursts) are hot enough to allow for breakout from the Hot CNO hydrogen burning cycles to the rapid proton capture (rp) process. An important breakout reaction sequence is 15O(α,γ)19Ne(p,γ)20Na and the 19Ne(p,γ)20Na reaction rate is expected to be dominated by a single resonance at 457 keV above the proton threshold in 20Na. The resonance strength and, hence, reaction rate depends strongly on whether this 20Na state at an excitation energy of 2647 keV has spin and parity of 1+ or 3+. Previous 20Mg (Jπ =0+) β+ decay experiments have relied almost entirely on searches for β-delayed proton emission from this resonance in 20Na to limit the log ft value and, hence, Jπ. However there is a non-negligible γ-ray branch expected that must also be limited experimentally to determine the log ft value and constrain Jπ. We have measured the β-delayed γ decay of 20Mg to complement previous β-delayed proton decay work and provide the first complete limit based on all energetically allowed decay channels through the 2647 keV state. Our limit confirms that a 1+ assignment for this state is highly unlikely.

Metastable phase in binary and ternary 12-carat gold alloys at low temperature

NASA Astrophysics Data System (ADS)

Lamiri, Imene; Abdelbaky, Mohammed S. M.; Hamana, Djamel; García-Granda, Santiago

2018-04-01

Low temperature phase transitions in 12-carat gold alloys have been investigated for binary Au-Cu and ternary Au-Cu-Ag compositions. The thermal analyses investigations using differential scanning calorimetry (DSC) and the dilatometry were performed in the 50–300 °C temperature range in order to detect the structural transformations. The thermal analyses were carried out on annealed samples at 700 °C for two hour followed by water quenching. They reveal an important new reaction for both used compositions and both thermal techniques confirm each other. This reaction has been assessed as pre-ordering reaction. SEM and STM imaging were performed on annealed samples at 700 °C for two hours and water quenched followed by a heating from room temperature up to the temperature of the new peaks obtained in the thermal study. The imaging reveals the relationship between the pre-ordering reaction and the surface aspect presented in the fact of dendrite precipitates. A series of SEM observation have been performed in order to follow the kinetic of the observed precipitates by the way of several series of heating up, from 140 to 220 °C for the binary composition and from 100 to 180 °C for the ternary composition. Furthermore, this study shows that the silver accelerates the ordering reaction.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schäfer, Gerhard

The current knowledge in the post-Newtonian (PN) dynamics and motion of non-spinning and spinning compact binaries will be presented based on the Arnowitt-Deser-Misner Hamiltonian approach to general relativity. The presentation will cover the binary dynamics with non-spinning components up to the 4PN order and for spinning binaries up to the next-to-next-to-leading order in the spin-orbit and spin-spin couplings. Radiation reaction will be treated for both non-spinning and spinning binaries. Explicit analytic expressions for the motion will be given, innermost stable circular orbits will be discussed.

Probing the N˜Z line via β decay

NASA Astrophysics Data System (ADS)

Oinonen, Markku

1999-11-01

This contribution reports several beta-decay studies performed at ISOLDE On-line Mass Separator at CERN recently for nuclei close to N=Z line. Beta decay of 58Zn provides a possibility to compare Gamow-Teller strength extracted from complementary beta-decay studies and charge-exchange reactions. Measurement on beta-decay half-life of 70Kr shows importance of experimental information in modelling the path of the astrophysical rp process. Decay of 71Kr is an example of a mirror beta decay and extends the systematics of these particular decays towards highly deformed region close to A=80.

How important is thermodynamics for identifying elementary flux modes?

PubMed Central

Peres, Sabine; Jolicœur, Mario; Moulin, Cécile

2017-01-01

We present a method for computing thermodynamically feasible elementary flux modes (tEFMs) using equilibrium constants without need of internal metabolite concentrations. The method is compared with the method based on a binary distinction between reversible and irreversible reactions. When all reactions are reversible, adding the constraints based on equilibrium constants reduces the number of elementary flux modes (EFMs) by a factor of two. Declaring in advance some reactions as irreversible, based on reliable biochemical expertise, can in general reduce the number of EFMs by a greater factor. But, even in this case, computing tEFMs can rule out some EFMs which are biochemically irrelevant. We applied our method to two published models described with binary distinction: the monosaccharide metabolism and the central carbon metabolism of Chinese hamster ovary cells. The results show that the binary distinction is in good agreement with biochemical observations. Moreover, the suppression of the EFMs that are not consistent with the equilibrium constants appears to be biologically relevant. PMID:28222104

Phenomenological study of exclusive binary light particle production from antiproton-proton annihilation at FAIR/PANDA

NASA Astrophysics Data System (ADS)

Ying, Wang

2016-08-01

Exclusive binary annihilation reactions induced by antiprotons of momentum from 1.5 to 15 GeV/c can be extensively investigated at FAIR/PANDA [1]. We are especially interested in the channel of charged pion pairs. Whereas this very probable channel constitutes the major background for other processes of interest in the PANDA experiment, it carries unique physical information on the quark content of proton, allowing to test different models (quark counting rules, statistical models,..). To study the binary reactions of light meson formation, we are developing an effective Lagrangian model based on Feynman diagrams which takes into account the virtuality of the exchanged particles. Regge factors [2] and form factors are introduced with parameters which may be adjusted on the existing data. We present preliminary results of our formalism for different reactions of light meson production leading to reliable predictions of cross sections, energy and angular dependencies in the PANDA kinematical range.

The influence of massive black hole binaries on the morphology of merger remnants

NASA Astrophysics Data System (ADS)

Bortolas, E.; Gualandris, A.; Dotti, M.; Read, J. I.

2018-06-01

Massive black hole (MBH) binaries, formed as a result of galaxy mergers, are expected to harden by dynamical friction and three-body stellar scatterings, until emission of gravitational waves (GWs) leads to their final coalescence. According to recent simulations, MBH binaries can efficiently harden via stellar encounters only when the host geometry is triaxial, even if only modestly, as angular momentum diffusion allows an efficient repopulation of the binary loss cone. In this paper, we carry out a suite of N-body simulations of equal-mass galaxy collisions, varying the initial orbits and density profiles for the merging galaxies and running simulations both with and without central MBHs. We find that the presence of an MBH binary in the remnant makes the system nearly oblate, aligned with the galaxy merger plane, within a radius enclosing 100 MBH masses. We never find binary hosts to be prolate on any scale. The decaying MBHs slightly enhance the tangential anisotropy in the centre of the remnant due to angular momentum injection and the slingshot ejection of stars on nearly radial orbits. This latter effect results in about 1 per cent of the remnant stars being expelled from the galactic nucleus. Finally, we do not find any strong connection between the remnant morphology and the binary hardening rate, which depends only on the inner density slope of the remnant galaxy. Our results suggest that MBH binaries are able to coalesce within a few Gyr, even if the binary is found to partially erase the merger-induced triaxiality from the remnant.

Nuclear Data Sheets for A = 230

DOE Office of Scientific and Technical Information (OSTI.GOV)

Browne, E.; Tuli, J. K.

The evaluators present in this publication spectroscopic data and level schemes from radioactive decay and nuclear reactions for all isobars with mass number A=230. This evaluation includes the first experimental evidence of 230Am, produced through the 197Au(40Ar,3n)234Bk (α decay to 230Am) reaction, E(40Ar)=188.4 MeV (2003MoZX).

The Trojan Horse method for nuclear astrophysics: Recent results for direct reactions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tumino, A.; Gulino, M.; Spitaleri, C.

2014-05-09

The Trojan Horse method is a powerful indirect technique to determine the astrophysical factor for binary rearrangement processes A+x→b+B at astrophysical energies by measuring the cross section for the Trojan Horse (TH) reaction A+a→B+b+s in quasi free kinematics. The Trojan Horse Method has been successfully applied to many reactions of astrophysical interest, both direct and resonant. In this paper, we will focus on direct sub-processes. The theory of the THM for direct binary reactions will be shortly presented based on a few-body approach that takes into account the off-energy-shell effects and initial and final state interactions. Examples of recent resultsmore » will be presented to demonstrate how THM works experimentally.« less

Double Charge Exchange Reactions and Double Beta Decay

NASA Astrophysics Data System (ADS)

Auerbach, N.

2018-05-01

The subject of this presentation is at the forefront of nuclear physics, namely double beta decay. In particular one is most interested in the neutrinoless process of double beta decay, when the decay proceeds without the emission of two neutrinos. The observation of such decay would mean that the lepton conservation symmetry is violated and that the neutrinos are of Majorana type, meaning that they are their own anti-particles. The life time of this process has two unknowns, the mass of the neutrino and the nuclear matrix element. Determining the nuclear matrix element and knowing the cross-section well will set limits on the neutrino mass. There is a concentrated effort among the nuclear physics community to calculate this matrix element. Usually these matrix elements are a very small part of the total strength of the transition operators involved in the process. There is no simple way to “calibrate” the nuclear double beta decay matrix element. The double beta decay is a double charge exchange process, therefore it is proposed that double charge exchange reactions using ion projectiles on nuclei that are candidates for double beta decay, will provide additional necessary information about the nuclear matrix elements.

Detailed spectroscopy of 110Cd: Evidence for weak mixing and the emergence of γ-soft behavior

NASA Astrophysics Data System (ADS)

Garrett, P. E.; Bangay, J.; Diaz Varela, A.; Ball, G. C.; Cross, D. S.; Demand, G. A.; Finlay, P.; Garnsworthy, A. B.; Green, K. L.; Hackman, G.; Hannant, C. D.; Jigmeddorj, B.; Jolie, J.; Kulp, W. D.; Leach, K. G.; Orce, J. N.; Phillips, A. A.; Radich, A. J.; Rand, E. T.; Schumaker, M. A.; Svensson, C. E.; Sumithrarachchi, C.; Triambak, S.; Warr, N.; Wong, J.; Wood, J. L.; Yates, S. W.

2012-10-01

A study of the β+-electron capture decay of 110In into levels of 110Cd is combined with a reanalysis of data from a previous study of 110Cd with the (n,n'γ) reaction with monoenergetic neutrons. The γγ coincidences from the 110In decay leads to many new assignments of γ rays observed in the (n,n'γ) reaction, permitting the observation of weak low-energy transitions, and setting stringent upper limits on unobserved decay branches. The uncertainties on many of the lifetimes from the (n,n'γ) reaction are significantly reduced, and limits are established for the lifetimes of levels too long for a direct measurement. The absence of enhanced transitions between the previously assigned phonon states and the deformed intruder states strongly suggests that mixing between the configurations is generally weak, refuting the strong-mixing scenario as an explanation of the decay pattern of the excited 0+ states in 110Cd. The decay pattern of the nonintruder states is suggestive of a γ-soft rotor, or O(6) nucleus, rather than a vibrational, or U(5), pattern. The existence of a four-particle-six-hole proton excitation in 110Cd is also suggested.

The birth of a supermassive black hole binary

NASA Astrophysics Data System (ADS)

Pfister, Hugo; Lupi, Alessandro; Capelo, Pedro R.; Volonteri, Marta; Bellovary, Jillian M.; Dotti, Massimo

2017-11-01

We study the dynamical evolution of supermassive black holes, in the late stage of galaxy mergers, from kpc to pc scales. In particular, we capture the formation of the binary, a necessary step before the final coalescence, and trace back the main processes causing the decay of the orbit. We use hydrodynamical simulations of galaxy mergers with different resolutions, from 20 pc down to 1 pc, in order to study the effects of the resolution on our results, remove numerical effects, and assess that resolving the influence radius of the orbiting black hole is a minimum condition to fully capture the formation of the binary. Our simulations include the relevant physical processes, namely star formation, supernova feedback, accretion on to the black holes and the ensuing feedback. We find that, in these mergers, dynamical friction from the smooth stellar component of the nucleus is the main process that drives black holes from kpc to pc scales. Gas does not play a crucial role and even clumps do not induce scattering or perturb the orbits. We compare the time needed for the formation of the binary to analytical predictions and suggest how to apply such analytical formalism to obtain estimates of binary formation times in lower resolution simulations.

Extrasolar binary planets. I. Formation by tidal capture during planet-planet scattering

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ochiai, H.; Nagasawa, M.; Ida, S., E-mail: nagasawa.m.ad@m.titech.ac.jp

2014-08-01

We have investigated (1) the formation of gravitationally bounded pairs of gas-giant planets (which we call 'binary planets') from capturing each other through planet-planet dynamical tide during their close encounters and (2) the subsequent long-term orbital evolution due to planet-planet and planet-star quasi-static tides. For the initial evolution in phase 1, we carried out N-body simulations of the systems consisting of three Jupiter-mass planets taking into account the dynamical tide. The formation rate of the binary planets is as much as 10% of the systems that undergo orbital crossing, and this fraction is almost independent of the initial stellarcentric semimajormore » axes of the planets, while ejection and merging rates sensitively depend on the semimajor axes. As a result of circularization by the planet-planet dynamical tide, typical binary separations are a few times the sum of the physical radii of the planets. After the orbital circularization, the evolution of the binary system is governed by long-term quasi-static tide. We analytically calculated the quasi-static tidal evolution in phase 2. The binary planets first enter the spin-orbit synchronous state by the planet-planet tide. The planet-star tide removes angular momentum of the binary motion, eventually resulting in a collision between the planets. However, we found that the binary planets survive the tidal decay for the main-sequence lifetime of solar-type stars (∼10 Gyr), if the binary planets are beyond ∼0.3 AU from the central stars. These results suggest that the binary planets can be detected by transit observations at ≳ 0.3 AU.« less

Simultaneous analysis of neutrinoless double beta decay and LHC pp-cross sections: limits on the left-right mixing angle

NASA Astrophysics Data System (ADS)

Civitarese, O.; Suhonen, J.; Zuber, K.

2015-09-01

The extension of the Standard Model of electroweak interactions, to accommodate massive neutrinos and/or right-handed currents, is one of the fundamental questions to answer in the cross-field of particle and nuclear physics. The consequences of such extensions would reflect upon nuclear decays, like the very exotic nuclear double-beta-decay, as well as upon high-energy proton-proton reactions of the type performed at the LHC accelerator. In this talk we shall address this question by looking at the results reported by the ATLAS and CMS collaborations, where the excitation and decay of a heavy-mass boson may be mediated by a heavy-mass neutrino in proton-proton reactions leading to two jets and two leptons, and by extracting limits on the left-right mixing, from the latest measurements of nuclear-double-beta decays reported by the GERDA and EXO collaborations.

Binary counting with chemical reactions.

PubMed

Kharam, Aleksandra; Jiang, Hua; Riedel, Marc; Parhi, Keshab

2011-01-01

This paper describes a scheme for implementing a binary counter with chemical reactions. The value of the counter is encoded by logical values of "0" and "1" that correspond to the absence and presence of specific molecular types, respectively. It is incremented when molecules of a trigger type are injected. Synchronization is achieved with reactions that produce a sustained three-phase oscillation. This oscillation plays a role analogous to a clock signal in digital electronics. Quantities are transferred between molecular types in different phases of the oscillation. Unlike all previous schemes for chemical computation, this scheme is dependent only on coarse rate categories for the reactions ("fast" and "slow"). Given such categories, the computation is exact and independent of the specific reaction rates. Although conceptual for the time being, the methodology has potential applications in domains of synthetic biology such as biochemical sensing and drug delivery. We are exploring DNA-based computation via strand displacement as a possible experimental chassis.

Physics with WASA-at-COSY

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schadmand, Susan

2010-12-28

The WASA detector facility is an internal experiment at the COoler SYnchrotron COSY in Juelich, Germany. The COSY accelerator provides proton and deuteron beams with momenta up to 3.7 GeV/c giving access to hadron physics including the strange quark sector. The WASA-at-COSY physics program focuses on light meson decays where rare decays are used to scrutinize symmetries and symmetry breaking. The structure of hadrons is probed with transition form factors and hadron spectroscopy while hadron dynamics is studied via reaction dynamics and few body reactions. Goals and status are reported with special emphasis on the meson Dalitz decays.

End-Member Formulation of Solid Solutions and Reactive Transport

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lichtner, Peter C.

2015-09-01

A model for incorporating solid solutions into reactive transport equations is presented based on an end-member representation. Reactive transport equations are solved directly for the composition and bulk concentration of the solid solution. Reactions of a solid solution with an aqueous solution are formulated in terms of an overall stoichiometric reaction corresponding to a time-varying composition and exchange reactions, equivalent to reaction end-members. Reaction rates are treated kinetically using a transition state rate law for the overall reaction and a pseudo-kinetic rate law for exchange reactions. The composition of the solid solution at the onset of precipitation is assumed tomore » correspond to the least soluble composition, equivalent to the composition at equilibrium. The stoichiometric saturation determines if the solid solution is super-saturated with respect to the aqueous solution. The method is implemented for a simple prototype batch reactor using Mathematica for a binary solid solution. Finally, the sensitivity of the results on the kinetic rate constant for a binary solid solution is investigated for reaction of an initially stoichiometric solid phase with an undersaturated aqueous solution.« less

Update and evaluation of decay data for spent nuclear fuel analyses

NASA Astrophysics Data System (ADS)

Simeonov, Teodosi; Wemple, Charles

2017-09-01

Studsvik's approach to spent nuclear fuel analyses combines isotopic concentrations and multi-group cross-sections, calculated by the CASMO5 or HELIOS2 lattice transport codes, with core irradiation history data from the SIMULATE5 reactor core simulator and tabulated isotopic decay data. These data sources are used and processed by the code SNF to predict spent nuclear fuel characteristics. Recent advances in the generation procedure for the SNF decay data are presented. The SNF decay data includes basic data, such as decay constants, atomic masses and nuclide transmutation chains; radiation emission spectra for photons from radioactive decay, alpha-n reactions, bremsstrahlung, and spontaneous fission, electrons and alpha particles from radioactive decay, and neutrons from radioactive decay, spontaneous fission, and alpha-n reactions; decay heat production; and electro-atomic interaction data for bremsstrahlung production. These data are compiled from fundamental (ENDF, ENSDF, TENDL) and processed (ESTAR) sources for nearly 3700 nuclides. A rigorous evaluation procedure of internal consistency checks and comparisons to measurements and benchmarks, and code-to-code verifications is performed at the individual isotope level and using integral characteristics on a fuel assembly level (e.g., decay heat, radioactivity, neutron and gamma sources). Significant challenges are presented by the scope and complexity of the data processing, a dearth of relevant detailed measurements, and reliance on theoretical models for some data.

Kinetics of Mn3+-oxalate formation and decay in reactions catalyzed by manganese peroxidase of Ceriporiopsis subvermispora

Treesearch

Ulises Urzua; Philip J. Kersten; Rafael Vicuna

1998-01-01

The kinetics of Mn3+- oxalate formation and decay were investigated in reactions catalyzed by manganese peroxidase (MnP) from the basiomycete Ceriporiopsis subvermispora in the absence of externally added hydrogen peroxide. A characteristic lag observed in the formation of this complex was shortened by glyoxylate or catalytic amounts of Mn3+ or hydrogen peroxide. MnP...

Nuclear Data Sheets for A = 230

DOE Office of Scientific and Technical Information (OSTI.GOV)

Browne, E.; Tuli, J.K.

The evaluators present in this publication spectroscopic data and level schemes from radioactive decay and nuclear reactions for all isobars with mass number A=230. This evaluation includes the first experimental evidence of {sup 230}Am, produced through the {sup 197}Au({sup 40}Ar,3n){sup 234}Bk ({alpha} decay to {sup 230}Am) reaction, E({sup 40}Ar)=188.4 MeV (2003MoZX).

Gravitational waves from remnant massive neutron stars of binary neutron star merger: Viscous hydrodynamics effects

NASA Astrophysics Data System (ADS)

Shibata, Masaru; Kiuchi, Kenta

2017-06-01

Employing a simplified version of the Israel-Stewart formalism of general-relativistic shear-viscous hydrodynamics, we explore the evolution of a remnant massive neutron star of binary neutron star merger and pay special attention to the resulting gravitational waveforms. We find that for the plausible values of the so-called viscous alpha parameter of the order 10-2 the degree of the differential rotation in the remnant massive neutron star is significantly reduced in the viscous time scale, ≲5 ms . Associated with this, the degree of nonaxisymmetric deformation is also reduced quickly, and as a consequence, the amplitude of quasiperiodic gravitational waves emitted also decays in the viscous time scale. Our results indicate that for modeling the evolution of the merger remnants of binary neutron stars we would have to take into account magnetohydrodynamics effects, which in nature could provide the viscous effects.

Effects of gravity reduction on phase equilibria. Part 1: Unary and binary isostructural solids

NASA Technical Reports Server (NTRS)

Larson, D. J., Jr.

1975-01-01

Analysis of the Skylab II M553 Experiment samples resulted in the hypothesis that the reduced gravity environment was altering the melting and solidification reactions. A theoretical study was conducted to define the conditions under which such alteration of phase relations is feasible, determine whether it is restricted to space processing, and, if so, ascertain which alloy systems or phase reactions are most likely to demonstrate such effects. Phase equilibria of unary and binary systems with a single solid phase (unary and isomorphous) were considered.

The formation mechanism of binary semiconductor nanomaterials: shared by single-source and dual-source precursor approaches.

PubMed

Yu, Kui; Liu, Xiangyang; Zeng, Qun; Yang, Mingli; Ouyang, Jianying; Wang, Xinqin; Tao, Ye

2013-10-11

One thing in common: The formation of binary colloidal semiconductor nanocrystals from single- (M(EEPPh2 )n ) and dual-source precursors (metal carboxylates M(OOCR)n and phosphine chalcogenides such as E=PHPh2 ) is found to proceed through a common mechanism. For CdSe as a model system (31) P NMR spectroscopy and DFT calculations support a reaction mechanism which includes numerous metathesis equilibriums and Se exchange reactions. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

A Nonequilibrium Rate Formula for Collective Motions of Complex Molecular Systems

NASA Astrophysics Data System (ADS)

Yanao, Tomohiro; Koon, Wang Sang; Marsden, Jerrold E.

2010-09-01

We propose a compact reaction rate formula that accounts for a non-equilibrium distribution of residence times of complex molecules, based on a detailed study of the coarse-grained phase space of a reaction coordinate. We take the structural transition dynamics of a six-atom Morse cluster between two isomers as a prototype of multi-dimensional molecular reactions. Residence time distribution of one of the isomers shows an exponential decay, while that of the other isomer deviates largely from the exponential form and has multiple peaks. Our rate formula explains such equilibrium and non-equilibrium distributions of residence times in terms of the rates of diffusions of energy and the phase of the oscillations of the reaction coordinate. Rapid diffusions of energy and the phase generally give rise to the exponential decay of residence time distribution, while slow diffusions give rise to a non-exponential decay with multiple peaks. We finally make a conjecture about a general relationship between the rates of the diffusions and the symmetry of molecular mass distributions.

The Beta-Delayed Proton and Gamma Decay of 27P for Nuclear Astrophysics

NASA Astrophysics Data System (ADS)

McCleskey, E.; Banu, A.; McCleskey, M.; Roeder, B.; Saastamoinen, A.; Spiridon, A.; Trache, L.; Tribble, R. E.; Davinson, T.; Doherty, D.; Lotay, G. J.; Wallace, J.; Woods, P. J.

2013-10-01

The main creation site of 26Al is currently under debate. The reactions for its creation or destruction are also not completely known. When 26Al is created in novae, the reaction chain is: 24Mg(p,γ)25Al(β + v)25Mg(p,γ)26Al, but this chain can be by-passed by another chain: 25Al(p,γ)26Si(p,γ)27P and it can also be destroyed directly. Another way to by-pass it is through 26mAl(p,γ)27Si* which is dominated by resonant capture. Using the Momentum Achromat Recoil Spectrometer (MARS) at the Texas A&M Cyclotron Institute and inverse kinematics, this destruction reaction was studied by the beta-delayed proton and gamma decay of 27P. Due to selection rules, states populated above the proton threshold in the compound system (27Si*) can decay to 26mAl, which are the states of interest for the capture reaction. James Madison University, VA, USA.

In situ monitoring of atomic layer controlled pore reduction in alumina tubular membranes using sequential surface reactions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Berland, B.S.; Gartland, I.P.; Ott, A.W.

1998-12-01

The pore diameter in alumina tubular membranes with an initial diameter of 50 {angstrom} was systematically reduced using the atomic layer controlled deposition of Al{sub 2}O{sub 3}. The Al{sub 2}O{sub 3} was deposited using sequential exposures of Al(CH{sub 3}){sub 3} (trimethylaluminum, TMA) and H{sub 2}O in an ABAB... binary reaction sequence. The pore diameter reduction was monitored using in situ N{sub 2} and Ar conductance measurements. The conductance, C = Q/{Delta}P, was measured using a mass flow controller to define a constant gas throughput, Q, and a pair of capacitance manometers to monitor the transmembrane pressure drop, {Delta}P. Conductance measurementsmore » were periodically obtained at 298 K as a function of AB binary reaction cycles. These conductance measurements were consistent with a pore diameter reduction from 50 {angstrom} to {approximately}5--10 {angstrom} at a rate of {approximately}2.5 {angstrom} for each AB cycle. Conductance measurements were also performed during the Al{sub 2}O{sub 3} deposition at 500 K after each half-reaction in the binary reaction sequence. These in situ conductance measurements demonstrate that the pore diameters in mesoporous membranes can be reduced to molecular dimensions with atomic layer control using sequential surface reactions. Poe diameters can be tailored for specific applications by varying the number of AB cycles and changing the nature of the terminating surface functional groups.« less

Spectroscopic binaries in the Solar Twin Planet Search program: from substellar-mass to M dwarf companions

NASA Astrophysics Data System (ADS)

dos Santos, Leonardo A.; Meléndez, Jorge; Bedell, Megan; Bean, Jacob L.; Spina, Lorenzo; Alves-Brito, Alan; Dreizler, Stefan; Ramírez, Iván; Asplund, Martin

2017-12-01

Previous studies on the rotation of Sun-like stars revealed that the rotational rates of young stars converge towards a well-defined evolution that follows a power-law decay. It seems, however, that some binary stars do not obey this relation, often by displaying enhanced rotational rates and activity. In the Solar Twin Planet Search program, we observed several solar twin binaries, and found a multiplicity fraction of 42 per cent ± 6 per cent in the whole sample; moreover, at least three of these binaries (HIP 19911, HIP 67620 and HIP 103983) clearly exhibit the aforementioned anomalies. We investigated the configuration of the binaries in the program, and discovered new companions for HIP 6407, HIP 54582, HIP 62039 and HIP 30037, of which the latter is orbited by a 0.06 M⊙ brown dwarf in a 1 m long orbit. We report the orbital parameters of the systems with well-sampled orbits and, in addition, the lower limits of parameters for the companions that only display a curvature in their radial velocities. For the linear trend binaries, we report an estimate of the masses of their companions when their observed separation is available, and a minimum mass otherwise. We conclude that solar twin binaries with low-mass stellar companions at moderate orbital periods do not display signs of a distinct rotational evolution when compared to single stars. We confirm that the three peculiar stars are double-lined binaries, and that their companions are polluting their spectra, which explains the observed anomalies.

Gravitational radiation from compact binary systems in screened modified gravity

NASA Astrophysics Data System (ADS)

Zhang, Xing; Liu, Tan; Zhao, Wen

2017-05-01

Screened modified gravity (SMG) is a kind of scalar-tensor theory with screening mechanisms, which can suppress the fifth force in dense regions and allow theories to evade the solar system and laboratory tests. In this paper, we investigate how the screening mechanisms in SMG affect the gravitational radiation damping effects, calculate in detail the rate of the energy loss due to the emission of tensor and scalar gravitational radiations, and derive their contributions to the change in the orbital period of the binary system. We find that the scalar radiation depends on the screened parameters and the propagation speed of scalar waves, and the scalar dipole radiation dominates the orbital decay of the binary system. For strongly self-gravitating bodies, all effects of scalar sector are strongly suppressed by the screening mechanisms in SMG. By comparing our results to observations of binary system PSR J 1738 +0333 , we place the stringent constraints on the screening mechanisms in SMG. As an application of these results, we focus on three specific models of SMG (chameleon, symmetron, and dilaton), and derive the constraints on the model parameters, respectively.

Recent Results from the WASA-at-COSY Experiment

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kupsc, Andrzej

2011-10-24

Studies of light meson decays are the key experiments for the WASA detector at COSY-Juelich. One of the world largest data samples of the {eta} meson decays have been recently collected in the pd {yields}{sup 3}He{eta} and in the pp {yields} pp{eta} reactions. The status of the analysis of various decay channels and the further plans for the light meson decay program are presented.

Signals of dynamical and statistical process from IMF-IMF correlation function

NASA Astrophysics Data System (ADS)

Pagano, E. V.; Acosta, L.; Auditore, L.; Baran, V.; Cap, T.; Cardella, G.; Colonna, M.; De Luca, S.; De Filippo, E.; Dell'Aquila, D.; Francalanza, L.; Gnoffo, B.; Lanzalone, G.; Lombardo, I.; Maiolino, C.; Martorana, N. S.; Norella, S.; Pagano, A.; Papa, M.; Piasecki, E.; Pirrone, S.; Politi, G.; Porto, F.; Quattrocchi, L.; Rizzo, F.; Rosato, E.; Russotto, P.; Siwek-Wilczyńska, K.; Trifiro, A.; Trimarchi, M.; Verde, G.; Vigilante, M.; Wilczyńsky, J.

2017-11-01

In this paper we briefly discuss about a novel application of the IMF-IMF correlation function to the physical case of binary massive projectile-like (PLF) splitting for dynamical and statistical breakup/fission in heavy ion collisions at Fermi energy. Theoretical simulations are also shown for comparisons with the data. These preliminary results have been obtained for the reverse kinematics reaction 124Sn + 64Ni at 35 AMeV that was studied using the forward part of CHIMERA detector. In that reaction a strong competition between a dynamical and a statistical components and its evolution with the charge asymmetry of the binary break up was already shown. In this work we show that the IMF-IMF correlation function can be used to pin down the timescale of the fragments production in binary fission-like phenomena. We also made simulations with the CoMDII model in order to compare to the experimental IMF-IMF correlation function. In future we plan to extend these studies to different reaction mechanisms and nuclear systems and to compare with different theoretical transport simulations.

Solute transport with multisegment, equilibrium-controlled, classical reactions: Problem solvability and feed forward method's applicability for complex segments of at most binary participants

USGS Publications Warehouse

Rubin, Jacob

1992-01-01

The feed forward (FF) method derives efficient operational equations for simulating transport of reacting solutes. It has been shown to be applicable in the presence of networks with any number of homogeneous and/or heterogeneous, classical reaction segments that consist of three, at most binary participants. Using a sequential (network type after network type) exploration approach and, independently, theoretical explanations, it is demonstrated for networks with classical reaction segments containing more than three, at most binary participants that if any one of such networks leads to a solvable transport problem then the FF method is applicable. Ways of helping to avoid networks that produce problem insolvability are developed and demonstrated. A previously suggested algebraic, matrix rank procedure has been adapted and augmented to serve as the main, easy-to-apply solvability test for already postulated networks. Four network conditions that often generate insolvability have been identified and studied. Their early detection during network formulation may help to avoid postulation of insolvable networks.

Investigating microbial transformations of soil organic matter: synthesizing knowledge from disparate fields to guide new experimentation

NASA Astrophysics Data System (ADS)

Billings, S. A.; Tiemann, L. K.; Ballantyne, F., IV; Lehmeier, C. A.; Min, K.

2015-04-01

Discerning why some soil organic matter (SOM) leaves soil profiles relatively quickly while other compounds, especially at depth, can be retained for decades to millennia is challenging for a multitude of reasons. Simultaneous with soil-specific advances, multiple other disciplines have enhanced their knowledge bases in ways potentially useful for future investigations of SOM decay. In this article, we highlight observations highly relevant for those investigating SOM decay and retention but often emanating from disparate fields and residing in literature seldom cited in SOM research. We focus on recent work in two key areas. First, we turn to experimental approaches using natural and artificial aquatic environments to investigate patterns of microbially mediated OM transformations as environmental conditions change, and highlight how aquatic microbial responses to environmental change can reveal processes likely important to OM decay and retention in soils. Second, we emphasize the importance of establishing intrinsic patterns of decay kinetics for purified substrates commonly found in soils to develop baseline rates. These decay kinetics - which represent the upper limit of the reaction rates - can then be compared to substrate decay kinetics observed in natural samples, which integrate intrinsic decay reaction rates and edaphic factors essential to the site under study but absent in purified systems. That comparison permits the site-specific factors to be parsed from the fundamental decay kinetics, an important advance in our understanding of SOM decay (and thus persistence) in natural systems. We then suggest ways in which empirical observations from aquatic systems and purified substrate-enzyme reaction kinetics can be used to advance recent theoretical efforts in SOM-focused research. Finally, we suggest how the observations in aquatic and purified substrate-enzyme systems could be used to help unravel the puzzles presented by oft-observed patterns of SOM characteristics with depth, as one example of the many perplexing SOM-related problems.

A precise measurement of the magnetic field in the corona of the black hole binary V404 Cygni

NASA Astrophysics Data System (ADS)

Dallilar, Yigit; Eikenberry, Stephen S.; Garner, Alan; Stelter, Richard D.; Gottlieb, Amy; Gandhi, Poshak; Casella, Piergiorgio; Dhillon, Vik S.; Marsh, Tom R.; Littlefair, Stuart P.; Hardy, Liam; Fender, Rob; Mooley, Kunal; Walton, Dominic J.; Fuerst, Felix; Bachetti, Matteo; Castro-Tirado, A. J.; Charcos, Miguel; Edwards, Michelle L.; Lasso-Cabrera, Nestor M.; Marin-Franch, Antonio; Raines, S. Nicholas; Ackley, Kendall; Bennett, John G.; Cenarro, A. Javier; Chinn, Brian; Donoso, H. Veronica; Frommeyer, Raymond; Hanna, Kevin; Herlevich, Michael D.; Julian, Jeff; Miller, Paola; Mullin, Scott; Murphey, Charles H.; Packham, Chris; Varosi, Frank; Vega, Claudia; Warner, Craig; Ramaprakash, A. N.; Burse, Mahesh; Punnadi, Sujit; Chordia, Pravin; Gerarts, Andreas; de Paz Martín, Héctor; Calero, María Martín; Scarpa, Riccardo; Acosta, Sergio Fernandez; Hernández Sánchez, William Miguel; Siegel, Benjamin; Pérez, Francisco Francisco; Viera Martín, Himar D.; Rodríguez Losada, José A.; Nuñez, Agustín; Tejero, Álvaro; Martín González, Carlos E.; Rodríguez, César Cabrera; Molgó, Jordi; Rodriguez, J. Esteban; Cáceres, J. Israel Fernández; Rodríguez García, Luis A.; Lopez, Manuel Huertas; Dominguez, Raul; Gaggstatter, Tim; Lavers, Antonio Cabrera; Geier, Stefan; Pessev, Peter; Sarajedini, Ata

2017-12-01

The binary system V404 Cygni consists of a red giant star orbiting a black hole. In 2015, a surge of accretion by the black hole caused the surrounding plasma to brighten suddenly for the first time since 1989, briefly becoming the brightest x-ray source in the sky. Dallilar et al. combined observations from radio, infrared, optical, and x-ray telescopes taken during the outburst. They compared how fast the flux decayed at each wavelength, which allowed them to constrain the size of the emitting region, determine that the plasma within it cooled through synchrotron radiation, and measure the magnetic field around the black hole.

Measurements of cross sections and decay properties of the isotopes of elements 112, 114, and 116 produced in the fusion reactions 233,238 U , 242Pu , and 248Cm + 48Ca

NASA Astrophysics Data System (ADS)

Oganessian, Yu. Ts.; Utyonkov, V. K.; Lobanov, Yu. V.; Abdullin, F. Sh.; Polyakov, A. N.; Shirokovsky, I. V.; Tsyganov, Yu. S.; Gulbekian, G. G.; Bogomolov, S. L.; Gikal, B. N.; Mezentsev, A. N.; Iliev, S.; Subbotin, V. G.; Sukhov, A. M.; Voinov, A. A.; Buklanov, G. V.; Subotic, K.; Zagrebaev, V. I.; Itkis, M. G.; Patin, J. B.; Moody, K. J.; Wild, J. F.; Stoyer, M. A.; Stoyer, N. J.; Shaughnessy, D. A.; Kenneally, J. M.; Wilk, P. A.; Lougheed, R. W.; Il'Kaev, R. I.; Vesnovskii, S. P.

2004-12-01

We have studied the dependence of the production cross sections of the isotopes 282,283 112 and 286,287 114 on the excitation energy of the compound nuclei 286112 and 290114 . The maximum cross section values of the xn -evaporation channels for the reaction 238U ( 48Ca ,xn) 286-x 112 were measured to be σ3n = 2.5 +1.8 -1.1 pb and σ4n = 0.6 +1.6 -0.5 pb ; for the reaction 242Pu ( 48Ca ,xn) 290-x 114 : σ2n ˜0.5 pb , σ3n = 3.6 +3.4 -1.7 pb , and σ4n = 4.5 +3.6 -1.9 pb . In the reaction 233U ( 48Ca ,2 4n) 277 279 112 at E*=34.9±2.2 MeV we measured an upper cross section limit of σxn ⩽0.6 pb . The observed shift of the excitation energy associated with the maximum sum evaporation residue cross section σER (E*) to values significantly higher than that associated with the calculated Coulomb barrier can be caused by the orientation of the deformed target nucleus in the entrance channel of the reaction. An increase of σER in the reactions of actinide targets with 48Ca is consistent with the expected increase of the survivability of the excited compound nucleus upon closer approach to the closed neutron shell N=184 . In the present work we detected 33 decay chains arising in the decay of the known nuclei 282112 , 283112 , 286114 , 287114 , and 288114 . In the decay of 287114 (α) → 283112 (α) → 279110 (SF) , in two cases out of 22, we observed decay chains of four and five sequential α transitions that end in spontaneous fission of 271Sg ( Tα/SF = 2.4 +4.3 -1.0 min) and 267Rf ( TSF ˜2.3 h) , longer decay chains than reported previously. We observed the new nuclide 292116 ( Tα = 18 +16 -6 ms, Eα =10.66±0.07 MeV) in the irradiation of the 248Cm target at a higher energy than in previous experiments. The observed nuclear decay properties of the nuclides with Z=104 118 are compared with theoretical nuclear mass calculations and the systematic trends of spontaneous fission properties. As a whole, they give a consistent pattern of decay of the 18 even- Z neutron-rich nuclides with Z=104 118 and N=163 177 . The experiments were performed with the heavy-ion beam delivered by the U400 cyclotron of the FLNR (JINR, Dubna) employing the Dubna gas-filled recoil separator.

Beta decay of exotic TZ = -1, -2 nuclei: the interesting case of 56Zn

NASA Astrophysics Data System (ADS)

Orrigo, S. E. A.; Rubio, B.; Fujita, Y.; Blank, B.; Gelletly, W.; Agramunt, J.; Algora, A.; Ascher, P.; Bilgier, B.; Cáceres, L.; Cakirli, R. B.; Fujita, H.; Ganioğlu, E.; Gerbaux, M.; Giovinazzo, J.; Grévy, S.; Kamalou, O.; Kozer, H. C.; Kucuk, L.; Kurtukian-Nieto, T.; Molina, F.; Popescu, L.; Rogers, A. M.; Susoy, G.; Stodel, C.; Suzuki, T.; Tamii, A.; Thomas, J. C.

2014-03-01

The β decay properties of the Tz = -2, 56Zn isotope and other proton-rich nuclei in the fp-shell have been investigated in an experiment performed at GANIL. The ions were produced in fragmentation reactions and implanted in a double-sided silicon strip detector surrounded by Ge EXOGAM clovers. Preliminary results for 56Zn are presented .The 56Zn decay proceeds mainly by β delayed proton emission, but β delayed gamma rays were also detected. Moreover, the exotic β delayed gamma-proton decay was observed for the first time. The 56Zn half-life and the energy levels populated in the 56Cu daughter have been determined. Knowledge of the gamma de-excitation of the mirror states in 56Co and the comparison with the results of the mirror charge exchange process, the 56Fe(3He,t) reaction (where 56Fe has Tz = +2), were important in the interpretation of the 56Zn decay data. The absolute Fermi and Gamow-Teller strengths have been deduced.

[Tooth decay and associated factors among adolescents in the north of the State of Minas Gerais, Brazil: a hierarchical analysis].

PubMed

Silveira, Marise Fagundes; Freire, Rafael Silveira; Nepomuceno, Marcela Oliveira; Martins, Andréa Maria Eleutério de Barros Lima; Marcopito, Luiz Francisco

2015-11-01

This is a cross-sectional population-based study (n = 763) conducted in the north of the State of Minas Gerais, which aimed to investigate the prevalence of tooth decay among adolescents and to identify the potential determinants of same. Probability sampling by conglomerates in multiple stages was used. Trained and calibrated professionals performed the data collection by means of intraoral examination and interviews in the previously selected households. In the analysis of the determinant factor for the presence of tooth decay, hierarchical binary logistic regression models were used. The prevalence of tooth decay, decayed, missing and filled teeth were 71.3%, 36.5%, 55.6% and 16%, respectively. The following averages were observed: DMFT (3.4 teeth), number of decayed (0.8 teeth), restored (2.4 teeth) and missing (0.2 teeth). The incidence of tooth decay was higher among adolescents who stated they were black/indigenous/brown (OR = 1.76), lived in crowded households (OR = 2.4), did not regularly visit or had never been to a dentist (OR = 1.9), used public or philanthropic services (OR = 1,8), had smoking habits (OR = 4.1), consumed alcohol (OR = 1.8), perceived their oral health negatively (OR = 5.9 and OR = 1.9) and had toothac in the last six months (OR = 2.0).

Organic alloy systems suitable for the investigation of regular binary and ternary eutectic growth

NASA Astrophysics Data System (ADS)

Sturz, L.; Witusiewicz, V. T.; Hecht, U.; Rex, S.

2004-09-01

Transparent organic alloys showing a plastic crystal phase were investigated experimentally using differential scanning calorimetry and directional solidification with respect to find a suitable model system for regular ternary eutectic growth. The temperature, enthalpy and entropy of phase transitions have been determined for a number of pure substances. A distinction of substances with and without plastic crystal phases was made from their entropy of melting. Binary phase diagrams were determined for selected plastic crystal alloys with the aim to identify eutectic reactions. Examples for lamellar and rod-like eutectic solidification microstructures in binary systems are given. The system (D)Camphor-Neopentylglycol-Succinonitrile is identified as a system that exhibits, among others, univariant and a nonvariant eutectic reaction. The ternary eutectic alloy close to the nonvariant eutectic composition solidifies with a partially faceted solid-liquid interface. However, by adding a small amount of Amino-Methyl-Propanediol (AMPD), the temperature of the nonvariant eutectic reaction and of the solid state transformation from plastic to crystalline state are shifted such, that regular eutectic growth with three distinct nonfaceted phases is observed in univariant eutectic reaction for the first time. The ternary phase diagram and examples for eutectic microstructures in the ternary and the quaternary eutectic alloy are given.

Neutrino nuclear responses for double beta decays and astro neutrinos by charge exchange reactions

NASA Astrophysics Data System (ADS)

Ejiri, Hiroyasu

2014-09-01

Neutrino nuclear responses are crucial for neutrino studies in nuclei. Charge exchange reactions (CER) are shown to be used to study charged current neutrino nuclear responses associated with double beta decays(DBD)and astro neutrino interactions. CERs to be used are high energy-resolution (He3 ,t) reactions at RCNP, photonuclear reactions via IAR at NewSUBARU and muon capture reactions at MUSIC RCNP and MLF J-PARC. The Gamow Teller (GT) strengths studied by CERs reproduce the observed 2 neutrino DBD matrix elements. The GT and spin dipole (SD) matrix elements are found to be reduced much due to the nucleon spin isospin correlations and the non-nucleonic (delta isobar) nuclear medium effects. Impacts of the reductions on the DBD matrix elements and astro neutrino interactions are discussed.

Water-based binary polyol process for the controllable synthesis of silver nanoparticles inhibiting human and foodborne pathogenic bacteria

USDA-ARS?s Scientific Manuscript database

The polyol process is a widely used strategy for producing nanoparticles from various reducible metallic precursors; however it requires a bulk polyol liquid reaction with additional protective agents at high temperatures. Here, we report a water-based binary polyol process using low concentrations ...

Measurement of the 169Tm(n,3n) 167Tm cross section and the associated branching ratios in the decay of 167Tm [Measurement of the 169Tm(n,3n) 167Tm cross section and the branching ratios in the decay of 167Tm

DOE PAGES

Champine, B.; Gooden, M. E.; Krishichayan, .; ...

2016-01-14

The cross section for the 169Tm(n,3n) 167Tm reaction was measured from 17 to 22 MeV using quasimonoenergetic neutrons produced by the 2H(d,n) 3He reaction. This energy range was studied to resolve the discrepancy between previous (n,3n) cross-section measurements. In addition, the absolute γ-ray branching ratios following the electron-capture decay of 167Tm were measured. Furthermore, these results provide more reliable nuclear data for an important diagnostic that is used at the National Ignition Facility to estimate the yield of reaction-in-flight neutrons produced via the inertial-confinement-fusion plasma in deuterium-tritium capsules.

Statistical gamma-ray decay studies at iThemba LABS

NASA Astrophysics Data System (ADS)

Wiedeking, M.; Bernstein, L. A.; Bleuel, D. L.; Brits, C. P.; Sowazi, K.; Görgen, A.; Goldblum, B. L.; Guttormsen, M.; Kheswa, B. V.; Larsen, A. C.; Majola, S. N. T.; Malatji, K. L.; Negi, D.; Nogwanya, T.; Siem, S.; Zikhali, B. R.

2017-09-01

A program to study the γ-ray decay from the region of high-level density has been established at iThemba LABS, where a high-resolution gamma-ray detector array is used in conjunction with silicon particle-telescopes. Results from two recent projects are presented: 1) The 74Ge(α,α'γ) reaction was used to investigate the Pygmy Dipole Resonance. The results were compared to (γ,γ') data and indicate that the dipole states split into mixed isospin and relatively pure isovector excitations. 2) Data from the 95Mo(d,p) reaction were used to develop a novel method for the determination of spins for low-lying discrete levels utilizing statistical γ-ray decay in the vicinity of the neutron separation energy. These results provide insight into the competition of (γ,n) and (γ,γ') reactions and highlights the need to correct for angular momentum barrier effects.

Heat and mass transfer in unsteady rotating fluid flow with binary chemical reaction and activation energy.

PubMed

Awad, Faiz G; Motsa, Sandile; Khumalo, Melusi

2014-01-01

In this study, the Spectral Relaxation Method (SRM) is used to solve the coupled highly nonlinear system of partial differential equations due to an unsteady flow over a stretching surface in an incompressible rotating viscous fluid in presence of binary chemical reaction and Arrhenius activation energy. The velocity, temperature and concentration distributions as well as the skin-friction, heat and mass transfer coefficients have been obtained and discussed for various physical parametric values. The numerical results obtained by (SRM) are then presented graphically and discussed to highlight the physical implications of the simulations.

Heat and Mass Transfer in Unsteady Rotating Fluid Flow with Binary Chemical Reaction and Activation Energy

PubMed Central

Awad, Faiz G.; Motsa, Sandile; Khumalo, Melusi

2014-01-01

In this study, the Spectral Relaxation Method (SRM) is used to solve the coupled highly nonlinear system of partial differential equations due to an unsteady flow over a stretching surface in an incompressible rotating viscous fluid in presence of binary chemical reaction and Arrhenius activation energy. The velocity, temperature and concentration distributions as well as the skin-friction, heat and mass transfer coefficients have been obtained and discussed for various physical parametric values. The numerical results obtained by (SRM) are then presented graphically and discussed to highlight the physical implications of the simulations. PMID:25250830

Reaction-mediated entropic effect on phase separation in a binary polymer system

NASA Astrophysics Data System (ADS)

Sun, Shujun; Guo, Miaocai; Yi, Xiaosu; Zhang, Zuoguang

2017-10-01

We present a computer simulation to study the phase separation behavior induced by polymerization in a binary system comprising polymer chains and reactive monomers. We examined the influence of interaction parameter between components and monomer concentration on the reaction-induced phase separation. The simulation results demonstrate that increasing interaction parameter (enthalpic effect) would accelerate phase separation, while entropic effect plays a key role in the process of phase separation. Furthermore, scanning electron microscopy observations illustrate identical morphologies as found in theoretical simulation. This study may enrich our comprehension of phase separation in polymer mixture.

Decay analysis of compound nuclei formed in reactions with exotic neutron-rich 9Li projectile and the synthesis of 217At* within the dynamical cluster-decay model

NASA Astrophysics Data System (ADS)

Kaur, Arshdeep; Kaushal, Pooja; Hemdeep; Gupta, Raj K.

2018-01-01

The decay of various compound nuclei formed via exotic neutron-rich 9Li projectile is studied within the dynamical cluster-decay model (DCM). Following the earlier work of one of us (RKG) and collaborators (M. Kaur et al. (2015) [1]), for an empirically fixed neck-length parameter ΔRemp, the only parameter in the DCM, at a given incident laboratory energy ELab, we are able to fit almost exactly the (total) fusion cross section σfus =∑x=16σxn for 9Li projectile on 208Pb and other targets, with σfus depending strongly on the target mass of the most abundant isotope and its (magic) shell structure. This result shows the predictable nature of the DCM. The neck-length parameter ΔRemp is fixed empirically for the decay of 217At* formed in 9Li + 208Pb reaction at a fixed laboratory energy ELab, and then the total fusion cross section σfus calculated for all other reactions using 9Li as a projectile on different targets. Apparently, this procedure could be used to predict σfus for 9Li-induced reactions where experimental data are not available. Furthermore, optimum choice of "cold" target-projectile combinations, forming "hot" compact configurations, are predicted for the synthesis of compound nucleus 217At* with 8Li + 209Pb as one of the target-projectile combination, or another (t , p) combination 48Ca + 169Tb, with a doubly magic 48Ca, as the best possibility.

Measurement of the 6He Decay Produced by the 9Be(n, α) 6 He Reaction

NASA Astrophysics Data System (ADS)

Cook, Katelyn; Coats, Micah; Yuly, Mark; Padalino, Stephen; Sangster, Craig; Regan, Sean

2016-10-01

The OMEGA laser at LLE is routinely used to implode gas-filled capsules to study light ion fusion reaction rates of interest to stellar nucleosynthesis. As a first step toward a possible measurement of the 3H(t,γ)6He radiative capture reaction, a detector system capable of measuring the 801 ms half-life of 6He has been developed and is being tested using 6He nuclei produced via the 9Be(n,α)6He reaction. Deuterons from the SUNY Geneseo tandem Pelletron produce neutrons in a thick deuterated polyethylene target via the 2H(d,n)3He reaction. These neutrons are allowed to strike a beryllium target placed in front of a silicon ΔE-E detector telescope, which is used to identify the β particles from 6He decay. Following an approximately five second long activation period, the beryllium sample is immediately counted for about five seconds. The pulse heights for each detector and the timestamp are recorded using a specially configured femtoDAQ acquision system and used to measure the decay curve. Funded in part by a Grant from the DOE through the Laboratory for Laser Energetics.

The first ICRANet catalog of binary-driven hypernovae

NASA Astrophysics Data System (ADS)

Pisani, G. B.; Ruffini, R.; Aimuratov, Y.; Bianco, C. L.; Karlica, M.; Kovacevic, M.; Moradi, R.; Muccino, M.; Penacchioni, A. V.; Primorac, D.; Rueda, J. A.; Wang, Y.

2018-01-01

In a series of recent publications, scientists from ICRANet, led by professor Remo Ruffini, have reached a novel comprehensive picture of gamma-ray bursts (GRBs) thanks to their development of a series of new theoretical approaches. Among those, the induced gravitational collapse (IGC) paradigm explains a class of energetic, long-duration GRBs associated with Ib/c supernovae (SN), recently named binary-driven hypernovae (BdHNe). BdHNe have a well defined set of observational features which allow to identify them. Among them, the main two are: 1) long duration of the GRB explosion, namely larger than 2 s in the rest frame; 2) a total energy, released in all directions by the GRB explosion, larger than 1052 ergs. A striking result is the observation, in the BdHNe sources, of a universal late time power-law decay in the X-rays luminosity after 104 s, with typical decaying slope of 1.5. This leads to the possible establishment of a new distance indicator having redshift up to z 8. Thanks to this novel theoretical and observational understanding, it was possible for ICRANet scientists to build the firstst BdHNe catalog, composed by the 345 BdHNe identified up to the end of 2016.

Long-term mass transfer and mixing-controlled reactions of a DNAPL plume from persistent residuals

NASA Astrophysics Data System (ADS)

Liu, Yuan; Illangasekare, Tissa H.; Kitanidis, Peter K.

2014-02-01

Understanding and being able to predict the long-term behavior of DNAPL (i.e., PCE and TCE) residuals after active remediation has ceased have become increasingly important as attention at many sites turns from aggressive remediation to monitored natural attenuation and long-term stewardship. However, plume behavior due to mass loading and reactions during these later phases is less studied as they involve large spatial and temporal scales. We apply both theoretical analysis and pore-scale simulations to investigate mass transfer from DNAPL residuals and subsequent reactions within the generated plume, and, in particular, to show the differences between early- and late-time behaviors of the plume. In the zone of entry of the DNAPL entrapment zone where the concentration boundary layer in the flowing groundwater has not fully developed, the pore-scale simulations confirm the past findings based on laboratory studies that the mass transfer increases as a power-law function of the Peclét number, and is enhanced due to reactions in the plume. Away from the entry zone and further down gradient, the long-term reactions are limited by the available additive and mixing in the porous medium, thereby behave considerably differently from the entry zone. For the reaction between the contaminant and an additive with intrinsic second-order bimolecular kinetics, the late-time reaction demonstrates a first-order decay macroscopically with respect to the mass of the limiting additive, not with respect to that of the contaminant. The late-time decay rate only depends on the intrinsic reaction rate and the solubility of the entrapped DNAPL. At the intermediate time, the additive decays exponentially with the square of time (t2), instead of time (t). Moreover, the intermediate decay rate also depends on the initial conditions, the spatial distribution of DNAPL residuals, and the effective dispersion coefficient.

Ionic fluids with r-6 pair interactions have power-law electrostatic screening

NASA Astrophysics Data System (ADS)

Kjellander, Roland; Forsberg, Björn

2005-06-01

The decay behaviour of radial distribution functions for large distances r is investigated for classical Coulomb fluids where the ions interact with an r-6 potential (e.g. a dispersion interaction) in addition to the Coulombic and the short-range repulsive potentials (e.g. a hard core). The pair distributions and the density-density (NN), charge-density (QN) and charge-charge (QQ) correlation functions are investigated analytically and by Monte Carlo simulations. It is found that the NN correlation function ultimately decays like r-6 for large r, just as it does for fluids of electroneutral particles interacting with an r-6 potential. The prefactor is proportional to the squared compressibility in both cases. The QN correlations decay in general like r-8 and the QQ correlations like r-10 in the ionic fluid. The average charge density around an ion decays generally like r-8 and the average electrostatic potential like r-6. This behaviour is in stark contrast to the decay behaviour for classical Coulomb fluids in the absence of the r-6 potential, where all these functions decay exponentially for large r. The power-law decays are, however, the same as for quantum Coulomb fluids. This indicates that the inclusion of the dispersion interaction as an effective r-6 interaction potential in classical systems yields the same decay behaviour for the pair correlations as in quantum ionic systems. An exceptional case is the completely symmetric binary electrolyte for which only the NN correlation has a power-law decay but not the QQ correlations. These features are shown by an analysis of the bridge function.

Decay properties and reaction dynamics of zirconium isotopes in the relativistic mean-field model

NASA Astrophysics Data System (ADS)

Panigrahi, M.; Panda, R. N.; Kumar, Bharat; Patra, S. K.

In the framework of relativistic mean-field theory, the ground state properties like binding energy, charge radius and quadrupole deformation parameter for various isotopes of zirconium from the valley of stability to drip-line region have been studied. The results are compared with the experimental data and we found reasonable agreement. The calculations are carried out for β-decay energy and β-decay half-life up to the drip-line. Total reaction and elastic differential cross-sections are also studied for few zirconium isotopes as projectiles with 12C as target, using different parameter sets namely NL3*, DD-ME2 and DD-PC1 in conjunction with Glauber model.

Superheavy nuclei from 48Ca-induced reactions

NASA Astrophysics Data System (ADS)

Oganessian, Yu. Ts.; Utyonkov, V. K.

2015-12-01

The discovery and investigation of the new region of superheavy nuclei at the DGFRS separator based on fusion reactions of 48Ca with 238U-249Cf target nuclei are reviewed. The production cross sections and summaries of the decay properties, including the results of the posterior experiments performed at the SHIP, BGS, and TASCA separators, as well as at the chemistry setups, are discussed and compared with the theoretical calculations and the systematic trends in the α-decay and spontaneous fission properties. The properties of the new nuclei, isotopes of elements 112-118, and their decay products demonstrate significant increases in the stability of the heaviest nuclei with increasing neutron number and closer approach to magic number N = 184.

A genetically optimized kinetic model for ethanol electro-oxidation on Pt-based binary catalysts used in direct ethanol fuel cells

NASA Astrophysics Data System (ADS)

Sánchez-Monreal, Juan; García-Salaberri, Pablo A.; Vera, Marcos

2017-09-01

A one-dimensional model is proposed for the anode of a liquid-feed direct ethanol fuel cell. The complex kinetics of the ethanol electro-oxidation reaction is described using a multi-step reaction mechanism that considers free and adsorbed intermediate species on Pt-based binary catalysts. The adsorbed species are modeled using coverage factors to account for the blockage of the active reaction sites on the catalyst surface. The reaction rates are described by Butler-Volmer equations that are coupled to a one-dimensional mass transport model, which incorporates the effect of ethanol and acetaldehyde crossover. The proposed kinetic model circumvents the acetaldehyde bottleneck effect observed in previous studies by incorporating CH3CHOHads among the adsorbed intermediates. A multi-objetive genetic algorithm is used to determine the reaction constants using anode polarization and product selectivity data obtained from the literature. By adjusting the reaction constants using the methodology developed here, different catalyst layers could be modeled and their selectivities could be successfully reproduced.

Development of the gateway recycling cloning system for multiple linking of expression cassettes in a defined order, and direction on gateway compatible binary vectors.

PubMed

Kimura, Tetsuya; Nakao, Akihide; Murata, Sachiko; Kobayashi, Yasuyuki; Tanaka, Yuji; Shibahara, Kenta; Kawazu, Tetsu; Nakagawa, Tsuyoshi

2013-01-01

We developed the Gateway recycling cloning system, which allows multiple linking of expression cassettes by multiple rounds of the Gateway LR reaction. Employing this system, the recycling donor vector pRED419 was subjected to the first LR reaction with an attR1-attR2 type destination vector. Then conversion vector pCON was subjected to an LR reaction to restore the attR1-attR2 site on the destination vector for the next cloning cycle. By repetition of these two simple steps, we linked four expression cassettes of a reporter gene in Gateway binary vector pGWB1, introduced the constructs into tobacco BY-2 cells, and observed the expression of transgenes.

Relaxation dynamics in a binary hard-ellipse liquid.

PubMed

Xu, Wen-Sheng; Sun, Zhao-Yan; An, Li-Jia

2015-01-21

Structural relaxation in binary hard spherical particles has been shown recently to exhibit a wealth of remarkable features when size disparity or mixture composition is varied. In this paper, we test whether or not similar dynamical phenomena occur in glassy systems composed of binary hard ellipses. We demonstrate via event-driven molecular dynamics simulation that a binary hard-ellipse mixture with an aspect ratio of two and moderate size disparity displays characteristic glassy dynamics upon increasing density in both the translational and the rotational degrees of freedom. The rotational glass transition density is found to be close to the translational one for the binary mixtures investigated. More importantly, we assess the influence of size disparity and mixture composition on the relaxation dynamics. We find that an increase of size disparity leads, both translationally and rotationally, to a speed up of the long-time dynamics in the supercooled regime so that both the translational and the rotational glass transition shift to higher densities. By increasing the number concentration of the small particles, the time evolution of both translational and rotational relaxation dynamics at high densities displays two qualitatively different scenarios, i.e., both the initial and the final part of the structural relaxation slow down for small size disparity, while the short-time dynamics still slows down but the final decay speeds up in the binary mixture with large size disparity. These findings are reminiscent of those observed in binary hard spherical particles. Therefore, our results suggest a universal mechanism for the influence of size disparity and mixture composition on the structural relaxation in both isotropic and anisotropic particle systems.

Role of higher-multipole deformations and noncoplanarity in the decay of the compound nucleus *220Th within the dynamical cluster-decay model

NASA Astrophysics Data System (ADS)

Hemdeep, Chopra, Sahila; Kaur, Arshdeep; Kaushal, Pooja; Gupta, Raj K.

2018-04-01

Background: The formation and decay of the *220Th compound nucleus (CN) formed via some entrance channels (16O+204Pb,40Ar+180Hf,48Ca+172Yb,82Se+138Ba ) at near barrier energies has been studied within the dynamical cluster-decay model (DCM) [Hemdeep et al. Phys. Rev. C 95, 014609 (2017), 10.1103/PhysRevC.95.044603], for quadrupole deformations (β2 i) and "optimum" orientations (θopt) of the two nuclei or decay fragments lying in the same plane (coplanar nuclei, Φ =0∘ ). Purpose: We aim to investigate the role of higher-multipole deformations, the octupole (β3 i) and hexadecupole (β4 i), and "compact" orientations (θc i) together with the noncoplanarity degree of freedom (Φc) in the noncompound nucleus (nCN) cross section, already observed in the above mentioned study with quadrupole deformations (β2 i) alone, the Φ =0∘ case. Methods: The dynamical cluster-decay model (DCM), based on the quantum mechanical fragmentation theory (QMFT), is used to analyze the decay channel cross sections σx n for various experimentally studied entrance channels. The parameter Ra (equivalently, the neck length Δ R in Ra=R1+R2+Δ R ), which fixes both the preformation and penetration paths, is used to best fit both unobserved (1 n ,2 n ) and observed (3 n -5 n ) decay channel cross sections, keeping the root-mean-square (r.m.s) deviation to the minimum, which allows us to predict the nCN effects, if any, and fusion-fission (ff) cross sections in various reactions at different CN excitation energies E*. Results: For the decay of CN *220Th, the mass fragmentation potential V (Ai ) and preformation yields P0( Ai ) show an asymmetric fission mass distribution, in agreement with one observed in experiments, independent of adding or not adding (β3 i,β4 i ), and irrespective of large changes (by 36° and 34°), respectively, in "compact" orientations θc i and noncoplanarity Φc, and also in the potential energy surface V (Ai ) in light mass (1 n -5 n ) decays. Whereas the 3 n - and 5 n -decay channels fit nearly exactly, i.e., they are always the pure CN decays, the 4 n -decay channel shows the presence of large (˜95 % ) nCN content whose magnitude in every case remains the same within <1 % and hence does not get modified, in contrast to our earlier studies of other CN. Also, the near constancy of best fitted Ra(≡Δ R ) with E*, and with an upper limiting value for reactions with magic nuclei as reaction partner(s), independent of the entrance channel nuclei, allows us to predict the decay channel cross sections σx n,x =3 -5 for 16O+204Pb reaction, whose sum (=∑35σx n ) fits the observed σER data nicely. Also, the variations of CN fusion/formation probability PC N and survival probability Psurv follow the required systematic behavior, giving credence to our DCM analysis. Conclusions: With the inclusion of higher-multipole deformations and "compact" noncoplanarity degree of freedom (Φc≠0 ), the results of our above-mentioned earlier study, using quadrupole deformation (β2 i) alone for coplanar (Φc=0 ) nuclei, remain the same; i.e., of the measured 3 n -5 n decay channels of CN *220Th, the 3 n and 5 n decays are always pure CN decays and the 4 n decay is mainly of nCN content σn CN, whose magnitude also remains constant (within <1 % ) under all approximations. Furthermore, the upper limiting value of the linear dependence of first turning point Ra on E* is shown to be a better choice for predicting the decay channel cross sections σx n for reactions like 16O+204Pb using magic nuclei, whose experimental determination will be a good test of our model.

Experimental survey of the production of α -decaying heavy elements in 238U+232Th reactions at 7.5-6.1 MeV/nucleon

NASA Astrophysics Data System (ADS)

Wuenschel, S.; Hagel, K.; Barbui, M.; Gauthier, J.; Cao, X. G.; Wada, R.; Kim, E. J.; Majka, Z.; Płaneta, R.; Sosin, Z.; Wieloch, A.; Zelga, K.; Kowalski, S.; Schmidt, K.; Ma, C.; Zhang, G.; Natowitz, J. B.

2018-06-01

The production of α -particle decaying heavy nuclei in reactions of 7.5-6.1 MeV/nucleon 238U +232Th was explored using an in-beam detection array composed of YAP scintillators and gas ionization chamber-Si telescopes. Comparisons of α energies and half-lives for the observed products with those of the previously known isotopes and with theoretically predicted values indicate the observation of a number of previously unreported α emitters. α -particle decay energies reaching as high as 12 MeV are observed. Many of these are expected to be from decay of previously unseen relatively neutron rich products. While the contributions of isomeric states require further exploration and specific isotope identifications need to be made, the production of heavy isotopes with quite high atomic numbers is suggested by the data.

Quantum-state-selective decay spectroscopy of 213Ra

NASA Astrophysics Data System (ADS)

Lorenz, Ch.; Sarmiento, L. G.; Rudolph, D.; Ward, D. E.; Block, M.; Heßberger, F. P.; Ackermann, D.; Andersson, L.-L.; Cortés, M. L.; Droese, C.; Dworschak, M.; Eibach, M.; Forsberg, U.; Golubev, P.; Hoischen, R.; Kojouharov, I.; Khuyagbaatar, J.; Nesterenko, D.; Ragnarsson, I.; Schaffner, H.; Schweikhard, L.; Stolze, S.; Wenzl, J.

2017-09-01

An experimental scheme combining the mass resolving power of a Penning trap with contemporary decay spectroscopy has been established at GSI Darmstadt. The Universal Linear Accelerator (UNILAC) at GSI Darmstadt provided a 48Ca beam impinging on a thin 170Er target foil. Subsequent to velocity filtering of reaction products in the Separator for Heavy Ion reaction Products (SHIP), the nuclear ground state of the 5 n evaporation channel 213Ra was mass-selected in SHIPTRAP, and the 213Ra ions were finally transferred into an array of silicon strip detectors surrounded by large composite germanium detectors. Based on comprehensive geant4 simulations and supported by theoretical calculations, the spectroscopic results call for a revision of the decay path of 213Ra, thereby exemplifying the potential of a combination of a mass-selective Penning trap device with a dedicated nuclear decay station and contemporary geant4 simulations.

Experimental data on ground- and excited-state properties for all nuclei with mass number A=144 have been compiled and evaluated. States populated in radioactive decay as well as in nuclear reactions have been considered. For these nuclei, level and decay schemes have been built, as well as tables of nuclear properties. This work supersedes the 1989 evaluation by J.K. Tuli (1989Tu02). Manuscripts published before December 2000 have been included in this work

NASA Astrophysics Data System (ADS)

Sonzogni, A. A.

2001-07-01

Experimental data on ground- and excited-state properties for all nuclei with mass number A = 144 have been compiled and evaluated. States populated in radioactive decay as well as in nuclear reactions have been considered. For these nuclei, level and decay schemes have been built, as well as tables of nuclear properties. This work supersedes the 1989 evaluation by J.K. Tuli (1989Tu02). Manuscripts published before December 2000 have been included in this work.

Tz=-1 →0 β decays of 54Ni,50Fe,46Cr, and 42Ti and comparison with mirror (3He,t ) measurements

NASA Astrophysics Data System (ADS)

Molina, F.; Rubio, B.; Fujita, Y.; Gelletly, W.; Agramunt, J.; Algora, A.; Benlliure, J.; Boutachkov, P.; Cáceres, L.; Cakirli, R. B.; Casarejos, E.; Domingo-Pardo, C.; Doornenbal, P.; Gadea, A.; Ganioǧlu, E.; Gascón, M.; Geissel, H.; Gerl, J.; Górska, M.; GrÈ©bosz, J.; Hoischen, R.; Kumar, R.; Kurz, N.; Kojouharov, I.; Susam, L. Amon; Matsubara, H.; Morales, A. I.; Oktem, Y.; Pauwels, D.; Pérez-Loureiro, D.; Pietri, S.; Podolyák, Zs.; Prokopowicz, W.; Rudolph, D.; Schaffner, H.; Steer, S. J.; Tain, J. L.; Tamii, A.; Tashenov, S.; Valiente-Dobón, J. J.; Verma, S.; Wollersheim, H.-J.

2015-01-01

We have studied the β decay of the Tz=-1 ,f7 /2 shell nuclei 54Ni,50Fe,46Cr, and 42Ti produced in fragmentation reactions. The proton separation energies in the daughter Tz=0 nuclei are relatively large (≈4 -5 MeV) so studies of the γ rays are essential. The experiments were performed at GSI as part of the Stopped-beam campaign with the RISING setup consisting of 15 Euroball Cluster Ge detectors. From the newly obtained high precision β -decay half-lives, excitation energies, and β branching ratios, we were able to extract Fermi and Gamow-Teller transition strengths in these β decays. With these improved results it was possible to compare in detail the Gamow-Teller (GT) transition strengths observed in beta decay including a sensitivity limit with the strengths of the Tz=+1 to Tz=0 transitions derived from high resolution (3He ,t ) reactions on the mirror target nuclei at RCNP, Osaka. The accumulated B (GT) strength obtained from both experiments looks very similar although the charge exchange reaction provides information on a broader energy range. Using the "merged analysis" one can obtain a full picture of the B (GT) over the full Qβ range. Looking at the individual transitions some differences are observed, especially for the weak transitions. Their possible origins are discussed.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wieselquist, William A.

SCALE’s general depletion, activation, and spent fuel source terms analysis capabilities are enabled through a family of modules related to the main ORIGEN depletion/irradiation/decay solver. The nuclide tracking in ORIGEN is based on the principle of explicitly modeling all available nuclides and transitions in the current fundamental nuclear data for decay and neutron-induced transmutation and relies on fundamental cross section and decay data in ENDF/B VII. Cross section data for materials and reaction processes not available in ENDF/B-VII are obtained from the JEFF-3.0/A special purpose European activation library containing 774 materials and 23 reaction channels with 12,617 neutron-induced reactions belowmore » 20 MeV. Resonance cross section corrections in the resolved and unresolved range are performed using a continuous-energy treatment by data modules in SCALE. All nuclear decay data, fission product yields, and gamma-ray emission data are developed from ENDF/B-VII.1 evaluations. Decay data include all ground and metastable state nuclides with half-lives greater than 1 millisecond. Using these data sources, ORIGEN currently tracks 174 actinides, 1149 fission products, and 974 activation products. The purpose of this chapter is to describe the stand-alone capabilities and underlying methodology of ORIGEN—as opposed to the integrated depletion capability it provides in all coupled neutron transport/depletion sequences in SCALE, as described in other chapters.« less

31Cl beta decay and the 30P31S reaction rate in nova nucleosynthesis

NASA Astrophysics Data System (ADS)

Bennett, Michael; Wrede, C.; Brown, B. A.; Liddick, S. N.; Pérez-Loureiro, D.; NSCL e12028 Collaboration

2016-03-01

The 30P31S reaction rate is critical for modeling the final isotopic abundances of ONe nova nucleosynthesis, identifying the origin of presolar nova grains, and calibrating proposed nova thermometers. Unfortunately, this rate is essentially experimentally unconstrained because the strengths of key 31S proton capture resonances are not known, due to uncertainties in their spins and parities. Using a 31Cl beam produced at the National Superconducting Cyclotron Laboratory, we have populated several 31S states for study via beta decay and devised a new decay scheme which includes updated beta feedings and gamma branchings as well as multiple states previously unobserved in 31Cl beta decay. Results of this study, including the unambiguous identification due to isospin mixing of a new l = 0 , Jπ = 3 /2+ 31S resonance directly in the middle of the Gamow Window, will be presented, and significance to the evaluation of the 30P31S reaction rate will be discussed. Work supported by U.S. Natl. Sci. Foundation (Grants No. PHY-1102511, PHY-1404442, PHY-1419765, and PHY-1431052); U.S. Dept. of Energy, Natl. Nucl. Security Administration (Award No. DE-NA0000979); Nat. Sci. and Eng. Research Council of Canada.

Studies of Elementary Reactions of Chemical Importance in the Atmospheres of Planets

NASA Technical Reports Server (NTRS)

Nesbitt, Fred L.

2001-01-01

The methyl self-reaction was studied at T = 298 K and 202 K and at three different pressures, P = 0.5, 1.0, and 2.1 Torr. The experimental measurements were performed in our discharge flow-mass spectrometer (DF-MS) apparatus. The methyl radicals were generated by the reaction of F with methane. Passing a mixture of molecular fluorine, F2, in helium through a microwave cavity generated the atomic fluorine reagent. The atomic F enters the flow tube through a rear port on the flow tube. The methane reagent enters the flow tube through a movable injector located coaxial in the flow tube. The decay of methyl radical signal was monitored at a mass/charge ratio (m/z) of 15 as a function of the injector distance. To minimize secondary chemistry from the reaction CH3 + F to CH2 + HF the initial [CH4](sub 0)/[F](sub 0) was above 37.0 and typically 100. This ensures a 1:1 relationship between initial [F] and [CH3]. A titration of F with excess Cl2 yields the initial [F](sub 0). Our experimental methodology to accurately measure the mass spectrometer scaling factor, i.e., the relationship between initial signal and [CH3](sub 0) has been improved. Now we measure the CH3 signal decay under exponential decay conditions at low initial [F](sub 0), 3x10(exp 11) molecule/cc, in the presence of Cl2. This minimizes the second-order decay contributed by the CH3 self-reaction and a simple extrapolation of the 1n(signal) vs time plot to t = 0 gives the initial signal. This provides the desired relationship between initial signal at 15 amu and [CH3](sub 0). The resulting calibration is then applied to the observed decay of the CH3 signal at high concentrations of CH3 assuming linearity of this scaling factor.

Discovery of Nearly Coherent Oscillations with a Frequency of approximately 567 Hz During Type I X-ray Bursts of the X-ray Transient and Eclipsing Binary X1658-298

NASA Technical Reports Server (NTRS)

Wijnands, Rudy; Strohmayer, Tod; Franco, Lucia M.; White, Nicholas E. (Technical Monitor)

2001-01-01

We report the discovery of nearly coherent oscillations with a frequency of approximately 567 Hz during type I X-ray bursts from the X-ray transient and eclipsing binary X1658-298. If these oscillations are directly related to the neutron star rotation, then the spin period of the neutron star in X1658-298 is approximately 1.8 ms. The oscillations can be present during the rise or decay phase of the bursts. Oscillations during the decay phase of the bursts show an increase in frequency of approximately 0.5-1 Hz. However, in one particular burst the oscillations reappear at the end of the decay phase at about 571.5 Hz. This represents an increase in oscillation frequency of about 5 Hz, which is the largest frequency change seen so far in a burst oscillation. It is unclear if such a large change can be accommodated by present models used to explain the frequency evolution of the oscillations. The oscillations at 571.5 Hz are unusually soft compared to the oscillations found at 567 Hz. We also observed several bursts during which the oscillations are detected at much lower significance or not at all. Most of these bursts happen during periods of X-ray dipping behavior, suggesting that the X-ray dipping might decrease the amplitude of the oscillations (although several complications exist with this simple picture). We discuss our discovery in the framework of the neutron star spin interpretation.

Tidal interactions of inspiraling compact binaries

NASA Technical Reports Server (NTRS)

Bildsten, Lars; Cutler, Curt

1992-01-01

We discuss the tidal interaction in neutron star-neutron star and neutron star-black hole binaries and argue that they will not be tidally locked during the gravitational inspiral. More specifically, we show that, for inspiraling neutron stars of mass greater than about 1.2 solar mass, the shortest possible tidal synchronization time exceeds the gravitational decay time, so that the neutron star cannot be tidally locked prior to tidal disruption, regardless of its internal viscosity. For smaller mass neutron stars, an implausibly large kinematic viscosity - nearly the speed of light times the stellar radius - is required for tidal locking. We also argue that the mass transfer which occurs when the neutron star reaches the tidal radius will be unstable in neutron star-black hole binaries, and the instability will destroy the neutron star in a few orbital periods. The implications of our work for the detection of these sources by LIGO and other gravitational wave observatories and for the gamma-ray burst scenarios of Paczynski (1986, 1991) are discussed.

Fundamental frequencies and resonances from eccentric and precessing binary black hole inspirals

NASA Astrophysics Data System (ADS)

Lewis, Adam G. M.; Zimmerman, Aaron; Pfeiffer, Harald P.

2017-06-01

Binary black holes which are both eccentric and undergo precession remain unexplored in numerical simulations. We present simulations of such systems which cover about 50 orbits at comparatively high mass ratios 5 and 7. The configurations correspond to the generic motion of a nonspinning body in a Kerr spacetime, and are chosen to study the transition from finite mass-ratio inspirals to point particle motion in Kerr. We develop techniques to extract analogs of the three fundamental frequencies of Kerr geodesics, compare our frequencies to those of Kerr, and show that the differences are consistent with self-force corrections entering at first order in mass ratio. This analysis also locates orbital resonances where the ratios of our frequencies take rational values. At the considered mass ratios, the binaries pass through resonances in one to two resonant cycles, and we find no discernible effects on the orbital evolution. We also compute the decay of eccentricity during the inspiral and find good agreement with the leading order post-Newtonian prediction.

Three-body affairs in the outer solar system

NASA Astrophysics Data System (ADS)

Funato, Yoko; Makino, Junichiro; Hut, Piet; Kokubo, Eiichiro; Kinoshita, Daisuke

Recent observations have revealed an unexpectedly high binary fraction among the Trans-Neptunian Objects (TNOs) that populate the Kuiper Belt. The TNO binaries are strikingly different from asteroid binaries in four respects: their frequency is an order of magnitude larger, the mass ratio of their components is closer to unity, and their orbits are wider and highly eccentric. Two explanations have been proposed for their formation, one assuming large numbers of massive bodies, and one assuming large numbers of light bodies. We argue that both assumptions are unwarranted, and we show how TNO binaries can be produced from a modest number of intermediate-mass bodies of the type predicted by the gravitational instability theory for the formation of planetesimals. We start with a TNO binary population similar to the asteroid binary population, but subsequently modified by three-body exchange reactions, a process that is far more efficient in the Kuiper belt, because of the much smaller tidal perturbations by the Sun. Our mechanism can naturally account for all four characteristics that distinguish TNO binaries from main-belt asteroid binaries.

Supermassive Black Holes and Galaxy Evolution

NASA Technical Reports Server (NTRS)

Merritt, D.

2004-01-01

Supermassive black holes appear to be generic components of galactic nuclei. The formation and growth of black holes is intimately connected with the evolution of galaxies on a wide range of scales. For instance, mergers between galaxies containing nuclear black holes would produce supermassive binaries which eventually coalesce via the emission of gravitational radiation. The formation and decay of these binaries is expected to produce a number of observable signatures in the stellar distribution. Black holes can also affect the large-scale structure of galaxies by perturbing the orbits of stars that pass through the nucleus. Large-scale N-body simulations are beginning to generate testable predictions about these processes which will allow us to draw inferences about the formation history of supermassive black holes.

Gamma rays from pulsar wind shock acceleration

NASA Technical Reports Server (NTRS)

Harding, Alice K.

1990-01-01

A shock forming in the wind of relativistic electron-positron pairs from a pulsar, as a result of confinement by surrounding material, could convert part of the pulsar spin-down luminosity to high energy particles through first order Fermi acceleration. High energy protons could be produced by this mechanism both in supernova remnants and in binary systems containing pulsars. The pion-decay gamma-rays resulting from interaction of accelerated protons with surrounding target material in such sources might be observable above 70 MeV with EGRET (Energetic Gamma-Ray Experimental Telescope) and above 100 GeV with ground-based detectors. Acceleration of protons and expected gamma-ray fluxes from SN1987A, Cyg X-3 type sources and binary pulsars are discussed.

Formation and decay analysis of Cd *48 98 ,104 isotopes in 40Ca20-induced reactions

NASA Astrophysics Data System (ADS)

Gautam, Manjeet Singh; Kaur, Amandeep; Sharma, Manoj K.

2015-11-01

We have analyzed the fusion dynamics of Ca4020+Ni 28 58 ,64 reactions by using the energy dependent Woods-Saxon potential (EDWSP) model and coupled channel model and subsequently the decay patterns of Cd *48 98 ,104 nuclei are governed via the dynamical cluster-decay model (DCM). The influence of intrinsic degrees of freedom of colliding pairs, such as low lying surface vibrations and neutron transfer channels, are entertained within the context of coupled channel calculations. Interestingly, the energy dependence in the Woods-Saxon potential induces barrier modification effects (barrier height, barrier position, barrier curvature) in a somewhat similar way as that for coupled channel approach, hence adequately explains the observed fusion dynamics of Ca4020+Ni 28 58 ,64 reactions. In addition, the decay analysis of compound nuclei formed in the fusion of Ca4020+Ni 28 58 ,64 reactions is investigated by using DCM. The calculations are done for quadrupole (β2) deformed fragments having optimum orientations for hot configurations. The experimental data for evaporation residues lying within the wide range of center of mass energy (Ec .m .) of 64 -88 MeV is nicely addressed using the collective clusterization approach of the DCM. The comparative analysis of decay profiles of Cd *48 98 ,104 is worked out by introducing angular momentum and temperature effects in the fragmentation potential and preformation factor.

ASCA Observations of the Barnard 209 Dark Cloud and an Intense X-Ray Flare on V773 Tauri

NASA Technical Reports Server (NTRS)

Skinner, Stephen L.; Guedel, Manuel; Koyama, Katsuji; Yamauchi, Shigeo

1997-01-01

ASCA (Advanced Satellite for Cosmology and Astrophysics) detected an intense X-ray flare on the weak-lined T Tauri star V773 Tau (=HD 283447) during a 30 ks observation of the Barnard 209 dark cloud in 1995 September. This star is a spectroscopic binary and shows signs of strong magnetic surface activity including a spot-modulated optical light curve. The flare was seen only during its decay phase but is still one of the strongest ever recorded from a T Tauri star with a peak luminosity L(sub x) = 10(exp 32.4) ergs/s (0.5-10 keV), a maximum temperature of at least 42 million K, and energy release of greater than 10(exp 37) ergs. A shorter ASCA observation taken five months later showed V773 Tau in a quiescent state (L(sub x)= 10(exp 31.0) ergs/s) and detected variable emission from the infrared binary IRAS 04113+2758. The differential emission measure (DEM) distribution during the V773 Tau flare shows a bimodal temperature structure that is almost totally dominated by hot plasma at an average temperature of approx. 37 million K. Using information from time-resolved spectra, we examine the flare decay in terms of solar flare models (cooling loops and two-ribbon flares) and also consider possible nonsolar behavior (interbinary flares, star-disk flares, and rotational X-ray modulation). Solar models are unable to reproduce the unusual convex-shaped X-ray light curve, which decays slowly over a timespan of at least 1 day. However, the light curve decay is accurately modeled as a sinusoid with an inferred X-ray period of 2.97 days, which is nearly identical to the optical rotation period(s) of the two K-type components. This provides tantalizing evidence that the flaring region was undergoing rotational occultation, but periodic X-ray variability is not yet proven since our ASCA observation spans only one-third of a rotation cycle.

Simultaneous Transformation of Commingled Trichloroethylene, Tetrachloroethylene, and 1,4-Dioxane by a Microbially Driven Fenton Reaction in Batch Liquid Cultures.

PubMed

Sekar, Ramanan; Taillefert, Martial; DiChristina, Thomas J

2016-11-01

Improper disposal of 1,4-dioxane and the chlorinated organic solvents trichloroethylene (TCE) and tetrachloroethylene (also known as perchloroethylene [PCE]) has resulted in widespread contamination of soil and groundwater. In the present study, a previously designed microbially driven Fenton reaction system was reconfigured to generate hydroxyl (HO˙) radicals for simultaneous transformation of source zone levels of single, binary, and ternary mixtures of TCE, PCE, and 1,4-dioxane. The reconfigured Fenton reaction system was driven by fed batch cultures of the Fe(III)-reducing facultative anaerobe Shewanella oneidensis amended with lactate, Fe(III), and contaminants and exposed to alternating anaerobic and aerobic conditions. To avoid contaminant loss due to volatility, the Fe(II)-generating, hydrogen peroxide-generating, and contaminant transformation phases of the microbially driven Fenton reaction system were separated. The reconfigured Fenton reaction system transformed TCE, PCE, and 1,4-dioxane either as single contaminants or as binary and ternary mixtures. In the presence of equimolar concentrations of PCE and TCE, the ratio of the experimentally derived rates of PCE and TCE transformation was nearly identical to the ratio of the corresponding HO˙ radical reaction rate constants. The reconfigured Fenton reaction system may be applied as an ex situ platform for simultaneous degradation of commingled TCE, PCE, and 1,4-dioxane and provides valuable information for future development of in situ remediation technologies. A microbially driven Fenton reaction system [driven by the Fe(III)-reducing facultative anaerobe S. oneidensis] was reconfigured to transform source zone levels of TCE, PCE, and 1,4-dioxane as single contaminants or as binary and ternary mixtures. The microbially driven Fenton reaction may thus be applied as an ex situ platform for simultaneous degradation of at least three (and potentially more) commingled contaminants. Additional targets for ex situ and in situ degradation by the microbially driven Fenton reaction developed in the present study include multiple combinations of environmental contaminants susceptible to attack by Fenton reaction-generated HO˙ radicals, including commingled plumes of 1,4-dioxane, pentachlorophenol (PCP), PCE, TCE, 1,1,2-trichloroethane (TCA), and perfluoroalkylated substances (PFAS). Copyright © 2016, American Society for Microbiology. All Rights Reserved.

Simultaneous Transformation of Commingled Trichloroethylene, Tetrachloroethylene, and 1,4-Dioxane by a Microbially Driven Fenton Reaction in Batch Liquid Cultures

PubMed Central

Sekar, Ramanan; Taillefert, Martial

2016-01-01

ABSTRACT Improper disposal of 1,4-dioxane and the chlorinated organic solvents trichloroethylene (TCE) and tetrachloroethylene (also known as perchloroethylene [PCE]) has resulted in widespread contamination of soil and groundwater. In the present study, a previously designed microbially driven Fenton reaction system was reconfigured to generate hydroxyl (HO˙) radicals for simultaneous transformation of source zone levels of single, binary, and ternary mixtures of TCE, PCE, and 1,4-dioxane. The reconfigured Fenton reaction system was driven by fed batch cultures of the Fe(III)-reducing facultative anaerobe Shewanella oneidensis amended with lactate, Fe(III), and contaminants and exposed to alternating anaerobic and aerobic conditions. To avoid contaminant loss due to volatility, the Fe(II)-generating, hydrogen peroxide-generating, and contaminant transformation phases of the microbially driven Fenton reaction system were separated. The reconfigured Fenton reaction system transformed TCE, PCE, and 1,4-dioxane either as single contaminants or as binary and ternary mixtures. In the presence of equimolar concentrations of PCE and TCE, the ratio of the experimentally derived rates of PCE and TCE transformation was nearly identical to the ratio of the corresponding HO˙ radical reaction rate constants. The reconfigured Fenton reaction system may be applied as an ex situ platform for simultaneous degradation of commingled TCE, PCE, and 1,4-dioxane and provides valuable information for future development of in situ remediation technologies. IMPORTANCE A microbially driven Fenton reaction system [driven by the Fe(III)-reducing facultative anaerobe S. oneidensis] was reconfigured to transform source zone levels of TCE, PCE, and 1,4-dioxane as single contaminants or as binary and ternary mixtures. The microbially driven Fenton reaction may thus be applied as an ex situ platform for simultaneous degradation of at least three (and potentially more) commingled contaminants. Additional targets for ex situ and in situ degradation by the microbially driven Fenton reaction developed in the present study include multiple combinations of environmental contaminants susceptible to attack by Fenton reaction-generated HO˙ radicals, including commingled plumes of 1,4-dioxane, pentachlorophenol (PCP), PCE, TCE, 1,1,2-trichloroethane (TCA), and perfluoroalkylated substances (PFAS). PMID:27542932

A pulse radiolysis study of the dynamics of ascorbic acid free radicals within a liposomal environment.

PubMed

Kobayashi, Kazuo; Seike, Yumiko; Saeki, Akinori; Kozawa, Takahiro; Takeuchi, Fusako; Tsubaki, Motonari

2014-10-06

The dynamics of free-radical species in a model cellular system are examined by measuring the formation and decay of ascorbate radicals within a liposome with pulse radiolysis techniques. Upon pulse radiolysis of an N2O-saturated aqueous solution containing ascorbate-loaded liposome vesicles, ascorbate radicals are formed by the reaction of OH(·) radicals with ascorbate in unilamellar vesicles exclusively, irrespective of the presence of vesicle lipids. The radicals are found to decay rapidly compared with the decay kinetics in an aqueous solution. The distinct radical reaction kinetics in the vesicles and in bulk solution are characterized, and the kinetic data are analyzed. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Isospin influence on the decay modes of compound nuclei produced in the 78, 86Kr + 40, 48Ca at 10 MeV/nucleon

NASA Astrophysics Data System (ADS)

Pirrone, S.; Politi, G.; Wieleczko, J. P.; Gnoffo, B.; De Filippo, E.; La Commara, M.; Russotto, P.; Trimarchi, M.; Vigilante, M.; Ademard, G.; Auditore, L.; Beck, C.; Bercenau, I.; Bonnet, E.; Borderie, B.; Cardella, G.; Chibihi, A.; Colonna, M.; D'Onofrio, A.; Frankland, J. D.; Lanzalone, G.; Lautesse, P.; Lebhertz, D.; Le Neidre, N.; Lombardo, I.; Mazurek, K.; Pagano, A.; Pagano, E. V.; Papa, M.; Piasecki, E.; Porto, F.; Quattrocchi, L.; Rizzo, F.; Spadaccini, G.; Trifirò, A.; Verde, G.

2017-09-01

The study of the decay modes competition of the compound systems produced in the collisions ^{78}{Kr} + ^{40}{Ca} and ^{86}{Kr} + ^{48}{Ca} at 10MeV/A is presented. In particular, the N / Z entrance channel influence on the decay paths of the compound systems, directly connected to the isospin influence, is investigated. The experiment was performed at the INFN Laboratori Nazionali del Sud (LNS) in Catania by using the 4 π multi-detector CHIMERA. Charge, mass, angular distributions and kinematical features of the reaction products were studied. The analysis shows some differences in the contribution arising from the various reaction mechanisms for the neutron-poor and neutron-rich systems.

Investigating microbial transformations of soil organic matter: synthesizing knowledge from disparate fields to guide new experimentation

NASA Astrophysics Data System (ADS)

Billings, S. A.; Tiemann, L. K.; Ballantyne, F., IV; Lehmeier, C.; Min, K.

2014-12-01

Investigators of soil organic matter (SOM) transformations struggle with a deceptively simple-sounding question: "Why does some SOM leave the soil profile relatively quickly, while other compounds, especially those at depth, appear to be retained on timescales ranging from the decadal to the millennial?" This question is important on both practical and academic levels, but addressing it is challenging for a multitude of reasons. Simultaneous with soil-specific advances, multiple other disciplines have enhanced their knowledge bases in ways potentially useful for future investigations of SOM decay. In this article, we highlight observations highly relevant for those investigating SOM decay and retention but often emanating from disparate fields and residing in literature seldom cited in SOM research. We focus on recent work in two key areas. First, we turn to experimental approaches using natural and artificial aquatic environments to investigate patterns of microbially-mediated OM transformations as environmental conditions change, and highlight how aquatic microbial responses to environmental change can reveal processes likely important to OM decay and retention in soils. Second, we emphasize the importance of establishing intrinsic patterns of decay kinetics for purified substrates commonly found in soils to develop baseline rates. These decay kinetics - which represent the upper limit of the reaction rates - can then be compared to substrate decay kinetics observed in natural samples, which integrate intrinsic decay reaction rates and edaphic factors essential to the site under study but absent in purified systems. That comparison permits the site-specific factors to be parsed from the fundamental decay kinetics, an important advance in our understanding of SOM decay (and thus persistence) in natural systems. We then suggest ways in which empirical observations from aquatic systems and purified enzyme-substrate reaction kinetics can be used to advance recent theoretical efforts in SOM-focused research. Finally, we suggest how the observations in aquatic and purified enzyme-substrate systems could be used to help unravel the puzzles presented by oft-observed patterns of SOM characteristics with depth, as one example of the many perplexing SOM-related problems.

A search for periodicity in the x ray spectrum of black hole candidate A0620-00

NASA Technical Reports Server (NTRS)

Clark, George W.; Plaks, Kenneth

1991-01-01

The archived data from the SAS-3 observations of the X-ray nova A0620-00, the best of the stellar blackhole candidates, were exhaustively examined for evidence of variable phenomena correlated with the orbital motion of the binary system of which it is a member. The original analysis of these data was completed before discovery of the binary companion and determination of the orbital period of the system. New interest was drawn to the task of a reexamination of the archive data by the recent discovery of the massive nature of the X-ray source through analysis of the Doppler variations and ellipsoidal light variations of the faint K-star companion by McClintock and Remillard. The archive research, carried out under the supervision of the principal investigator, was the topic of the thesis submitted to the MIT Department of Physics by Kenneth Plaks in partial fulfillment of the requirements for the degree of Master of Science. Plaks' effort was focused on the elimination of fluctuations in the data due to errors in attitude solutions and other extraneous causes. The first products of his work were long-term light curves of the X-ray intensities in the various energy channels as functions of time during the time from outbursts in August 1975 to quiescence approximately 6 months later. These curves, are refined versions of the preliminary results published in 1976 (Matilsky et al. 1976). Smooth exponentials were fitted to these long term light curves to provide the basis for detrending the data, thereby permitting a calculation of residuals derived by subtracting the fitted curve from the data. The residuals were then analyzed by Fourier analysis to search for variations with the period of the binary orbit, namely 7.75 hours. No evidence of an orbital periodicity was found. However, the refined light curve provides a much clearer picture of the outburst and subsequent decay of the X-ray luminosity. In fact, there were two outbursts, each followed by an exponential decay with similar time constants of about 25 days. Previous evidence of a three-oscillation variation with a 7.8 day period were confirmed. Substantial theoretical effort has been devoted to attempts to account for the decay characteristics as the result of the gradual eating up of an accretion disk by a stellar-mass blackhole (e.g., Huang and Wheeler 1989). The improved decay curves will provide significant new constraints on the theoretical analyses.

Neutron-deficient superheavy nuclei obtained in the 240Pu+48Ca reaction

NASA Astrophysics Data System (ADS)

Utyonkov, V. K.; Brewer, N. T.; Oganessian, Yu. Ts.; Rykaczewski, K. P.; Abdullin, F. Sh.; Dmitriev, S. N.; Grzywacz, R. K.; Itkis, M. G.; Miernik, K.; Polyakov, A. N.; Roberto, J. B.; Sagaidak, R. N.; Shirokovsky, I. V.; Shumeiko, M. V.; Tsyganov, Yu. S.; Voinov, A. A.; Subbotin, V. G.; Sukhov, A. M.; Karpov, A. V.; Popeko, A. G.; Sabel'nikov, A. V.; Svirikhin, A. I.; Vostokin, G. K.; Hamilton, J. H.; Kovrizhnykh, N. D.; Schlattauer, L.; Stoyer, M. A.; Gan, Z.; Huang, W. X.; Ma, L.

2018-01-01

We present new results from investigations of the 240Pu+48Ca reaction at a projectile energy of 250 MeV. Three new decay chains of 285Fl were detected with decay properties mostly consistent with those measured in earlier studies. An additional chain was observed where the nuclei may decay through energy levels different from those of the other six chains registered so far. The cross section of the 240Pu(48Ca,3 n )285Fl reaction was measured to be 0 .58-0.33+0.60pb , which is a factor of about 4-5 lower than that measured in the previous experiment at 245 MeV beam energy [V. K. Utyonkov et al., Phys. Rev. C 92, 034609 (2015)., 10.1103/PhysRevC.92.034609], consistent with expectations. The origin of an additional chain consisting of a recoil, α particle, and fission event is analyzed. The assignment of 25 short-lived SF events observed in this experiment is also discussed.

Does Compound Nucleus remember its Isospin- An Evidence from the Fission Widths

NASA Astrophysics Data System (ADS)

Garg, Swati; Jain, Ashok Kumar

2018-05-01

We present an evidence of isospin effects in nuclear fission by comparing the fission widths for reactions involving different isospin states of the same compound nucleus (CN). Yadrovsky [1] suggested this possibility in 1975. Yadrovsky obtained the fission widths for two reaction data sets, namely 206Pb(α,f) and 209Bi(p,f), both leading to same CN, and concluded that "a nucleus remembers the isospin value of the nuclear states leading to fission". We obtain the fission decay widths for both the T0 + ½ and T0 - ½ states of CN by using two appropriate reaction data sets. We then compare the fission widths for the two isospin states of CN. More specifically, we have chosen the combination of 206Pb(α,f) and 209Bi(p,f) same as presented in Yadrovsky's paper [1] in this study. A significant difference between the ratios of fission decay widths to total decay widths for different isospin values suggests that isospin plays an important role in fission.

Excited state intramolecular charge transfer reaction in binary mixtures of water and tertiary butanol (TBA): alcohol mole fraction dependence.

PubMed

Pradhan, Tuhin; Ghoshal, Piue; Biswas, Ranjit

2008-02-07

The excited state intramolecular charge transfer reaction of 4-(1-azetidinyl)benzonitrile (P4C) has been studied in water-tertiary butanol (TBA) mixtures at different alcohol mole fractions by using steady state and time-resolved fluorescence spectroscopy. The ratio between the areas under the locally excited (LE) and charge transferred (CT) emission bands is found to exhibit a sharp rise at alcohol mole fraction approximately 0.04, a value at which several thermodynamic properties of this mixture is known to show anomalous change due to the enhancement of H-bonding network. The radiative rate associated with the LE emission also shows a maximum at this TBA mole fraction. Although the structural transition from the water-like tetrahedral network to the alcohol-like chain is reflected in the red shift of the absorption spectrum up to TBA mole fraction approximately 0.10, the emission bands (both LE and CT) show the typical nonideal alcohol mole fraction dependence at all TBA mole fractions. Quantum yield, CT radiative rate as well as transition moments also exhibit a nonideal alcohol mole fraction dependence. The time-resolved emission decay of P4C has been found to be biexponential at all TBA mole fractions, regardless of emission collection around either the LE or the CT bands. The time constant associated with the slow component (tau(slow)) shows a minimum at TBA mole fraction approximately 0.04, whereas such a minimum for the fast time constant, tau(fast) (representing the rate of LE --> CT conversion reaction) is not observed. The nonobservation of the minimum in tau(fast) might be due to the limited time resolution employed in our experiments.

Nanostructured Platinum Alloys for Use as Catalyst Materials

NASA Technical Reports Server (NTRS)

Narayan, Sri R. (Inventor); Hays, Charles C. (Inventor)

2015-01-01

A series of binary and ternary Pt-alloys, that promote the important reactions for catalysis at an alloy surface; oxygen reduction, hydrogen oxidation, and hydrogen and oxygen evolution. The first two of these reactions are essential when applying the alloy for use in a PEMFC.

Nanostructured Platinum Alloys for Use as Catalyst Materials

NASA Technical Reports Server (NTRS)

Hays, Charles C. (Inventor); Narayan, Sri R. (Inventor)

2013-01-01

A series of binary and ternary Pt-alloys, that promote the important reactions for catalysis at an alloy surface; oxygen reduction, hydrogen oxidation, and hydrogen and oxygen evolution. The first two of these reactions are essential when applying the alloy for use in a PEMFC.

Velocity autocorrelation function in supercooled liquids: Long-time tails and anomalous shear-wave propagation.

PubMed

Peng, H L; Schober, H R; Voigtmann, Th

2016-12-01

Molecular dynamic simulations are performed to reveal the long-time behavior of the velocity autocorrelation function (VAF) by utilizing the finite-size effect in a Lennard-Jones binary mixture. Whereas in normal liquids the classical positive t^{-3/2} long-time tail is observed, we find in supercooled liquids a negative tail. It is strongly influenced by the transfer of the transverse current wave across the period boundary. The t^{-5/2} decay of the negative long-time tail is confirmed in the spectrum of VAF. Modeling the long-time transverse current within a generalized Maxwell model, we reproduce the negative long-time tail of the VAF, but with a slower algebraic t^{-2} decay.

Selective protected state preparation of coupled dissipative quantum emitters

PubMed Central

Plankensteiner, D.; Ostermann, L.; Ritsch, H.; Genes, C.

2015-01-01

Inherent binary or collective interactions in ensembles of quantum emitters induce a spread in the energy and lifetime of their eigenstates. While this typically causes fast decay and dephasing, in many cases certain special entangled collective states with minimal decay can be found, which possess ideal properties for spectroscopy, precision measurements or information storage. We show that for a specific choice of laser frequency, power and geometry or a suitable configuration of control fields one can efficiently prepare these states. We demonstrate this by studying preparation schemes for strongly subradiant entangled states of a chain of dipole-dipole coupled emitters. The prepared state fidelity and its entanglement depth is further improved via spatial excitation phase engineering or tailored magnetic fields. PMID:26549501

Di-lepton yield from the decay of excited 28Si states

NASA Astrophysics Data System (ADS)

Bacelar, J. C.; Buda, A.; Bałanda, A.; Krasznahorkay, A.; van der Ploeg, H.; Sujkowski, Z.; van der Woude, A.

1994-03-01

The first dilepton yield measurements from excited nuclear states obtained with a new Positron-Electron Pair Spectroscopic Instrument (PEPSI) are reported. Nuclear states in 28Si, with an initial excitation energy E∗ = 50 MeV, were populated via the isospin T = 0 reaction 4He + 24Mg and the mixed-isospin 3He + 25Mg reaction. In both reactions the dilepton (e +e -) and photon decay yields were measured concurrently. An excess of counts in the e +e - spectrum, over the converted photon yield, is observed in the energy region above 15 MeV. An analyses is discussed whereby the observed excess counts are assumed to represent the isoscalar E0 strength in excited nuclear states.

Calculation of Formation and Decay of Heavy Compound Nuclei

NASA Astrophysics Data System (ADS)

Cherepanov, E. A.

2001-04-01

The report describes a method for calculating fusion and decay probabilities in reactions leading to the production of transfermium elements. The competition between quasi-fission and fussion is described on the basis of the Dinuclear System Concept (DNSC). The both competition between fusion and quasi-fission and statistical decay of heavy highly fissionable excited compound nuclei is described in an approach based on the Monte-Carlo method.

NICER and MAXI Observations of Two Large X-ray Flares from RS CVn Binaries

NASA Astrophysics Data System (ADS)

Drake, Stephen A.; Hamaguchi, Kenji; Corcoran, Michael Francis; Iwakiri, Wataru; Sasaki, Ryo; Kawai, Hiroki; Tsuboi, Yohko; Enoto, Teruaki; NICER Science Team

2018-01-01

NICER has observed two giant X-ray flares on the active binary systems, GT Mus and UX Ari, in response to their detections by the MAXI all-sky X-ray monitor onboard the ISS, with a delay of about a day in each case. The large effective area of the NICER X-ray optics means that high signal-to-noise spectra with more than 200,000 counts were obtained in relatively short exposures totaling less than an hour in each set of observations.MAXI detected a transient of 5.5 x 10^-10 erg/s/cm2 at the position of the active RS CVn binary GT Mus (G5/8 III + ?) early on 2017 July 19. NICER started its observations about 1 day later, and intermittently monitored the decay for the next 2.5 days, accumulating about 1,600 seconds exposure. The NICER light curve shows a smooth, gradual flux decline by a factor of two for the first 2 days, followed by an apparent flattening in the last half day. The dominant plasma temperature remained at ~40 million K during this period, suggesting an ongoing continuous heating during the decay phase.NICER also followed up another MAXI-detected flare in October 2017, this one from the nearby active system, UX Ari. NICER's X-ray spectrum shows clear neon and oxygen lines, while the emissionfrom iron ions is not as prominent as it is in most flares, implying an abundance of only ~10% solar which is significantly lower than previous inferred coronal Fe abundances for this star, although this result is dependent on the NICER gain correction.

Cross Section Measurements of the 76Ge (n ,n' γ) Reaction

NASA Astrophysics Data System (ADS)

Crider, B. P.; Peters, E. E.; Prados-Estévez, F. M.; Ross, T. J.; McEllistrem, M. T.; Yates, S. W.; Vanhoy, J. R.

2013-10-01

Neutrinoless double-beta decay (0 νββ) is a topic of great current interest and, as such, is the focus of several experiments and international collaborations. Two of these experiments, Majorana and GERDA, are seeking evidence of 0 νββ in the decay of 76Ge, where the signal would appear as a sharp peak in the energy spectrum at the Q-value of the reaction plus a small amount of recoil energy, or 2039 keV. Due to the high sensitivity of such a measurement, knowledge of background lines is critical. A study of 76Ga β- decay into 76Ge revealed a 2040.70(25)-keV transition from the 3951.70(14)-keV level, which, if populated, could potentially be a background line of concern. In addition to β- decay from 76Ga, a potential population mechanism could be cosmic-ray-induced inelastic neutron scattering. Measurements of the neutron-induced cross section of the 3951.70-keV level have been performed utilizing the 76 Ge (n ,n' γ) reaction at the University of Kentucky at neutron energies ranging from 4.3 to 4.9 MeV. This material is based upon work is supported by the U.S. National Science Foundation under grant no. PHY-0956310.

Measuring nuclear reaction cross sections to extract information on neutrinoless double beta decay

NASA Astrophysics Data System (ADS)

Cavallaro, M.; Cappuzzello, F.; Agodi, C.; Acosta, L.; Auerbach, N.; Bellone, J.; Bijker, R.; Bonanno, D.; Bongiovanni, D.; Borello-Lewin, T.; Boztosun, I.; Branchina, V.; Bussa, M. P.; Calabrese, S.; Calabretta, L.; Calanna, A.; Calvo, D.; Carbone, D.; Chávez Lomelí, E. R.; Coban, A.; Colonna, M.; D'Agostino, G.; De Geronimo, G.; Delaunay, F.; Deshmukh, N.; de Faria, P. N.; Ferraresi, C.; Ferreira, J. L.; Finocchiaro, P.; Fisichella, M.; Foti, A.; Gallo, G.; Garcia, U.; Giraudo, G.; Greco, V.; Hacisalihoglu, A.; Kotila, J.; Iazzi, F.; Introzzi, R.; Lanzalone, G.; Lavagno, A.; La Via, F.; Lay, J. A.; Lenske, H.; Linares, R.; Litrico, G.; Longhitano, F.; Lo Presti, D.; Lubian, J.; Medina, N.; Mendes, D. R.; Muoio, A.; Oliveira, J. R. B.; Pakou, A.; Pandola, L.; Petrascu, H.; Pinna, F.; Reito, S.; Rifuggiato, D.; Rodrigues, M. R. D.; Russo, A. D.; Russo, G.; Santagati, G.; Santopinto, E.; Sgouros, O.; Solakci, S. O.; Souliotis, G.; Soukeras, V.; Spatafora, A.; Torresi, D.; Tudisco, S.; Vsevolodovna, R. I. M.; Wheadon, R. J.; Yildirin, A.; Zagatto, V. A. B.

2018-02-01

Neutrinoless double beta decay (0vββ) is considered the best potential resource to access the absolute neutrino mass scale. Moreover, if observed, it will signal that neutrinos are their own anti-particles (Majorana particles). Presently, this physics case is one of the most important research “beyond Standard Model” and might guide the way towards a Grand Unified Theory of fundamental interactions. Since the 0vββ decay process involves nuclei, its analysis necessarily implies nuclear structure issues. In the NURE project, supported by a Starting Grant of the European Research Council (ERC), nuclear reactions of double charge-exchange (DCE) are used as a tool to extract information on the 0vββ Nuclear Matrix Elements. In DCE reactions and ββ decay indeed the initial and final nuclear states are the same and the transition operators have similar structure. Thus the measurement of the DCE absolute cross-sections can give crucial information on ββ matrix elements. In a wider view, the NUMEN international collaboration plans a major upgrade of the INFN-LNS facilities in the next years in order to increase the experimental production of nuclei of at least two orders of magnitude, thus making feasible a systematic study of all the cases of interest as candidates for 0vββ.

Black Hole-Neutron Star Mergers as Central Engines of Gamma-Ray Bursts.

PubMed

Janka; Eberl; Ruffert; Fryer

1999-12-10

Hydrodynamic simulations of the merger of stellar mass black hole-neutron star binaries are compared with mergers of binary neutron stars. The simulations are Newtonian but take into account the emission and back-reaction of gravitational waves. The use of a physical nuclear equation of state allows us to include the effects of neutrino emission. For low neutron star-to-black hole mass ratios, the neutron star transfers mass to the black hole during a few cycles of orbital decay and subsequent widening before finally being disrupted, whereas for ratios near unity the neutron star is destroyed during its first approach. A gas mass between approximately 0.3 and approximately 0.7 M middle dot in circle is left in an accretion torus around the black hole and radiates neutrinos at a luminosity of several times 1053 ergs s-1 during an estimated accretion timescale of about 0.1 s. The emitted neutrinos and antineutrinos annihilate into e+/- pairs with efficiencies of 1%-3% and rates of up to approximately 2x1052 ergs s-1, thus depositing an energy Enunu&d1; less, similar1051 ergs above the poles of the black hole in a region that contains less than 10-5 M middle dot in circle of baryonic matter. This could allow for relativistic expansion with Lorentz factors around 100 and is sufficient to explain apparent burst luminosities Lgamma approximately Enunu&d1;&solm0;&parl0;fOmegatgamma&parr0; up to several times 1053 ergs s-1 for burst durations tgamma approximately 0.1-1 s, if the gamma emission is collimated in two moderately focused jets in a fraction fOmega=2deltaOmega&solm0;&parl0;4pi&parr0; approximately 1&solm0;100-(1/10) of the sky.

Three-dimensional simulations of the interaction between the nova ejecta, accretion disk, and companion star

NASA Astrophysics Data System (ADS)

Figueira, Joana; José, Jordi; García-Berro, Enrique; Campbell, Simon W.; García-Senz, Domingo; Mohamed, Shazrene

2018-05-01

Context. Classical novae are thermonuclear explosions hosted by accreting white dwarfs in stellar binary systems. Material piles up on top of the white dwarf star under mildly degenerate conditions, driving a thermonuclear runaway. The energy released by the suite of nuclear processes operating at the envelope, mostly proton-capture reactions and β+-decays, heats the material up to peak temperatures ranging from 100 to 400 MK. In these events, about 10-3-10-7 M⊙, enriched in CNO and, sometimes, other intermediate-mass elements (e.g., Ne, Na, Mg, and Al) are ejected into the interstellar medium. Aims: To date, most of the efforts undertaken in the modeling of classical nova outbursts have focused on the early stages of the explosion and ejection, ignoring the interaction of the ejecta, first with the accretion disk orbiting the white dwarf and ultimately with the secondary star. Methods: A suite of 3D, smoothed-particle hydrodynamics (SPH) simulations of the interaction between the nova ejecta, accretion disk, and stellar companion were performed to fill this gap; these simulations were aimed at testing the influence of the model parameters—that is, the mass and velocity of the ejecta, mass and the geometry of the accretion disk—on the dynamical and chemical properties of the system. Results: We discuss the conditions that lead to the disruption of the accretion disk and to mass loss from the binary system. In addition, we discuss the likelihood of chemical contamination of the stellar secondary induced by the impact with the nova ejecta and its potential effect on the next nova cycle. Movies showing the full evolution of several models are available online at http://https://www.aanda.org and at http://www.fen.upc.edu/users/jjose/Downloads.html

Synthesis, Decay Properties, and Identification of Superheavy Nuclei Produced in 48Ca-induced Reactions

NASA Astrophysics Data System (ADS)

Oganessian, Yu. Ts.; Utyonkov, V. K.; Lobanov, Yu. V.; Abdullin, F. Sh.; Polyakov, A. N.; Sagaidak, R. N.; Shirokovsky, I. V.; Tsyganov, Yu. S.; Voinov, A. A.; Iliev, S.; Subbotin, V. G.; Sukhov, A. M.; Gulbekian, G. G.; Bogomolov, S. L.; Gikal, B. N.; Mezentsev, A. N.; Subotic, K.; Zagrebaev, V. I.; Itkis, M. G.; Moody, K. J.; Henderson, R. A.; Patin, J. B.; Shaughnessy, D. A.; Stoyer, M. A.; Stoyer, N. J.; Wilk, P. A.; Kenneally, J. M.; Landrum, J. H.; Wild, J. F.; Lougheed, R. W.

2007-10-01

Thirty-four new nuclides with Z = 104-116, 118 and N = 161-177 have been synthesized in the complete-fusion reactions of 238U, 237Np, 242,244Pu, 243Am, 245,248Cm, and 249Cf targets with 48Ca beams. The masses of evaporation residues were identified through measurements of the excitation functions of the xn-evaporation channels and from cross bombardments. The decay properties of the new nuclei agree with those of previously known heavy nuclei and with predictions from different theoretical models. A discussion of self-consistent interpretations of all observed decay chains originating from the parent isotopes 282,283112, 282113, 286-289114, 287,288115, 290-293116, and 294118 is presented. Decay energies and lifetimes of the neutron-rich superheavy nuclei as well as their production cross sections indicate a considerable increase in the stability of nuclei with the approach to the theoretically predicted nuclear shells with N = 184 and Z = 114.

Synthesis, Decay Properties, and Identification of Superheavy Nuclei Produced in 48CA-INDUCED Reactions

NASA Astrophysics Data System (ADS)

Oganessian, Yu. Ts.; Utyonkov, V. K.; Lobanov, Yu. V.; Abdullin, F. Sh.; Polyakov, A. N.; Sagaidak, R. N.; Shirokovsky, I. V.; Tsyganov, Yu. S.; Voinov, A. A.; Iliev, S.; Subbotin, V. G.; Sukhov, A. M.; Gulbekian, G. G.; Bogomolov, S. L.; Gikal, B. N.; Mezentsev, A. N.; Subotic, K.; Zagrebaev, V. I.; Itkis, M. G.; Moody, K. J.; Henderson, R. A.; Patin, J. B.; Shaughnessy, D. A.; Stoyer, M. A.; Stoyer, N. J.; Wilk, P. A.; Kenneally, J. M.; Landrum, J. H.; Wild, J. F.; Lougheed, R. W.

2008-04-01

Thirty-four new nuclides with Z = 104-116, 118 and N = 161-177 have been synthesized in the complete-fusion reactions of 238U, 237Np, 242,244Pu, 243Am, 245,248Cm, and 249Cf targets with 48Ca beams. The masses of evaporation residues were identified through measurements of the excitation functions of the xn-evaporation channels and from cross bombardments. The decay properties of the new nuclei agree with those of previously known heavy nuclei and with predictions from different theoretical models. A discussion of self-consistent interpretations of all observed decay chains originating from the parent isotopes 282,283112, 282113, 286-289114, 287,288115, 290-293116, and 294118 is presented. Decay energies and lifetimes of the neutron-rich superheavy nuclei as well as their production cross sections indicate a considerable increase in the stability of nuclei with the approach to the theoretically predicted nuclear shells with N = 184 and Z = 114.

Alpha decay properties of the semi-magic nucleus 219Np

NASA Astrophysics Data System (ADS)

Yang, H. B.; Ma, L.; Zhang, Z. Y.; Yang, C. L.; Gan, Z. G.; Zhang, M. M.; Huang, M. H.; Yu, L.; Jiang, J.; Tian, Y. L.; Wang, Y. S.; Wang, J. G.; Liu, Z.; Liu, M. L.; Duan, L. M.; Zhou, S. G.; Ren, Z. Z.; Zhou, X. H.; Xu, H. S.; Xiao, G. Q.

2018-02-01

The semi-magic nucleus 219Np was produced in the fusion reaction 187Re(36Ar, 4n)219Np at the gas-filled recoil separator SHANS (Spectrometer for Heavy Atoms and Nuclear Structure). A fast electronics system based on waveform digitizers was used in the data acquisition and the sampled pulses were processed by digital algorithms. The reaction products were identified using spatial and time correlations between the implants and subsequent α decays. According to the observed α-decay chain, an energy of Eα = 9039 (40) keV and a half-life of T1/2 =0.15-0.07 + 0.72 ms were determined for 219Np. The deduced proton binding energy of 219Np fits well into the systematics, which gives another evidence of that there is no sub-shell closure at Z = 92. The influence of the N = 126 shell closure on the stability of Np isotopes is discussed within the framework of α-decay reduced widths.

ϕ-meson photoproduction on hydrogen in the neutral decay mode

NASA Astrophysics Data System (ADS)

Seraydaryan, H.; Amaryan, M. J.; Gavalian, G.; Baghdasaryan, H.; Weinstein, L.; Adhikari, K. P.; Adikaram, D.; Aghasyan, M.; Anderson, M. D.; Pereira, S. Anefalos; Avakian, H.; Ball, J.; Baltzell, N. A.; Battaglieri, M.; Batourine, V.; Bedlinskiy, I.; Bennett, R. P.; Biselli, A. S.; Bono, J.; Boiarinov, S.; Briscoe, W. J.; Brooks, W. K.; Bültmann, S.; Burkert, V. D.; Carman, D. S.; Celentano, A.; Chandavar, S.; Collins, P.; Contalbrigo, M.; Cortes, O.; Crede, V.; D'Angelo, A.; Dashyan, N.; De Vita, R.; De Sanctis, E.; Deur, A.; Djalali, C.; Doughty, D.; Dugger, M.; Dupre, R.; Fassi, L. El; Eugenio, P.; Fedotov, G.; Fegan, S.; Fersch, R.; Fleming, J. A.; Gevorgyan, N.; Giovanetti, K. L.; Girod, F. X.; Goetz, J. T.; Gohn, W.; Golovatch, E.; Gothe, R. W.; Griffioen, K. A.; Guidal, M.; Guler, N.; Guo, L.; Hafidi, K.; Hakobyan, H.; Hanretty, C.; Harrison, N.; Heddle, D.; Hicks, K.; Ho, D.; Holtrop, M.; Hyde, C. E.; Ilieva, Y.; Ireland, D. G.; Ishkhanov, B. S.; Isupov, E. L.; Jo, H. S.; Joo, K.; Keller, D.; Khandaker, M.; Kim, A.; Kim, W.; Klein, F. J.; Koirala, S.; Kubarovsky, A.; Kubarovsky, V.; Kuhn, S. E.; Kuleshov, S. V.; Lewis, S.; Livingston, K.; Lu, H. Y.; MacGregor, I. J. D.; Martinez, D.; Mayer, M.; McKinnon, B.; Mineeva, T.; Mirazita, M.; Mokeev, V.; Montgomery, R. A.; Moutarde, H.; Munevar, E.; Camacho, C. Munoz; Nadel-Turonski, P.; Nasseripour, R.; Niccolai, S.; Niculescu, I.; Osipenko, M.; Ostrovidov, A. I.; Pappalardo, L. L.; Paremuzyan, R.; Park, K.; Park, S.; Pasyuk, E.; Phelps, E.; Phillips, J. J.; Pisano, S.; Pogorelko, O.; Pozdniakov, S.; Price, J. W.; Protopopescu, D.; Puckett, A. J. R.; Rimal, D.; Ripani, M.; Ritchie, B. G.; Rizzo, A.; Rosner, G.; Rossi, P.; Sabatié, F.; Saini, M. S.; Salgado, C.; Schott, D.; Schumacher, R. A.; Seder, E.; Sharabian, Y. G.; Smith, G. D.; Sober, D. I.; Sokhan, D.; Stepanyan, S.; Stoler, P.; Strakovsky, I. I.; Strauch, S.; Tang, W.; Taylor, C. E.; Tian, Ye; Tkachenko, S.; Ungaro, M.; Vineyard, M. F.; Voskanyan, H.; Voutier, E.; Walford, N. K.; Watts, D. P.; Weinstein, L. B.; Wood, M. H.; Zachariou, N.; Zana, L.; Zhang, J.; Zhao, Z. W.; CLAS Collaboration

2014-05-01

We report the first measurement of the photoproduction cross section of the ϕ meson in its neutral decay mode in the reaction γp →pϕ(KSKL). The experiment was performed with a tagged photon beam of energy 1.6≤Eγ≤3.6 GeV incident on a liquid hydrogen target of the CLAS spectrometer at the Thomas Jefferson National Accelerator Facility. The pϕ final state is identified via reconstruction of KS in the invariant mass of two oppositely charged pions and by requiring the missing particle in the reaction γp →pKSX to be KL. The presented results significantly enlarge the existing data on ϕ photoproduction. These data, combined with the data from the charged decay mode, will help to constrain different mechanisms of ϕ photoproduction.

First-order reactant in homogeneous turbulence before the final period of decay. [contaminant fluctuations in chemical reaction

NASA Technical Reports Server (NTRS)

Kumar, P.; Patel, S. R.

1974-01-01

A method is described for studying theoretically the concentration fluctuations of a dilute contaminate undergoing a first-order chemical reaction. The method is based on Deissler's (1958) theory for homogeneous turbulence for times before the final period, and it follows the approach used by Loeffler and Deissler (1961) to study temperature fluctuations in homogeneous turbulence. Four-point correlation equations are obtained; it is assumed that terms containing fifth-order correlation are very small in comparison with those containing fourth-order correlations, and can therefore be neglected. A spectrum equation is obtained in a form which can be solved numerically, yielding the decay law for the concentration fluctuations in homogeneous turbulence for the period much before the final period of decay.

Discovery of orbital decay in SMC X-1

NASA Technical Reports Server (NTRS)

Levine, A.; Rappaport, S.; Boynton, P.; Deeter, J.; Nagase, F.

1992-01-01

The results are reported of three observations of the binary X ray pulsar SMC X-1 with the Ginga satellite. Timing analyses of the 0.71 s X ray pulsations yield Doppler delay curves which, in turn, provide the most accurate determination of the SMC X-1 orbital parameters available to date. The orbital phase of the 3.9 day orbit is determined in May 1987, Aug. 1988, and Aug. 1988 with accuracies of 11, 1, and 3.5 s, respectively. These phases are combined with two previous determinations of the orbital phase to yield the rate of change in the orbital period: P sub orb/P sub orb = (-3.34 + or - 0.023) x 10(exp -6)/yr. An interpretation of this measurement and the known decay rate for the orbit of Cen X-3 is made in the context of tidal evolution. Finally, a discussion is presented of the relation among the stellar evolution, orbital decay, and neutron star spinup time scales for the SMC X-1 system.

All-sky monitor observations of the decay of A0620-00 (Nova monocerotis 1975)

NASA Technical Reports Server (NTRS)

Kaluzienski, L. J.; Holt, S. S.; Boldt, E. A.; Serlemitsos, P. J.

1976-01-01

The All-Sky X-ray Monitor onboard Ariel 5 has observed the 3-6 keV decline of the bright transient X-ray source A0620-00 on a virtually continuous basis during the period September 1975 - March 1976. The source behavior on timescales 100 minutes is characterized by smooth, exponential decays interrupted by substantial increases in October and February. The latter increase was an order-of-magnitude rise above the extrapolated exponential fall-off, and was followed by a final rapid decline. Upper limits of 2.5% and 10% were found for any periodicities in the range 0d.2 - 10d during the early and later decay phases, respectively. A probable correlation between the optical and 3-6 keV emission from A0620-00 was noted, effectively ruling out models involving traditional optical novae in favor of Roche-lobe overflow in a binary system. The existing data on the transient X-ray sources is consistent with two distinct luminosity-lifetime classes of these objects.

Electrical and optical properties of binary CNx nanocone arrays synthesized by plasma-assisted reaction deposition.

PubMed

Liu, Xujun; Guan, Leilei; Fu, Xiaoniu; Zhao, Yu; Wu, Jiada; Xu, Ning

2014-03-21

Light-absorbing and electrically conductive binary CNx nanocone (CNNC) arrays have been fabricated using a glow discharge plasma-assisted reaction deposition method. The intact CNNCs with amorphous structure and central nickel-filled pipelines could be vertically and neatly grown on nickel-covered substrates according to the catalyst-leading mode. The morphologies and composition of the as-grown CNNC arrays can be well controlled by regulating the methane/nitrogen mixture inlet ratio, and their optical absorption and resistivity strongly depend on their morphologies and composition. Beside large specific surface area, the as-grown CNNC arrays demonstrate high wideband absorption, good conduction, and nice wettability to polymer absorbers.

Binary collision rates of relativistic thermal plasmas. I Theoretical framework

NASA Technical Reports Server (NTRS)

Dermer, C. D.

1985-01-01

Binary collision rates for arbitrary scattering cross sections are derived in the case of a beam of particles interacting with a Maxwell-Boltzmann (MB) plasma, or in the case of two MB plasmas interacting at generally different temperatures. The expressions are valid for all beam energies and plasma temperatures, from the nonrelativistic to the extreme relativistic limits. The calculated quantities include the reaction rate, the energy exchange rate, and the average rate of change of the squared transverse momentum component of a monoenergetic particle beam as a result of scatterings with particles of a MB plasma. Results are specialized to elastic scattering processes, two-temperature reaction rates, or the cold plasma limit, reproducing previous work.

Nuclear Forensics and Radiochemistry: Reaction Networks

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rundberg, Robert S.

In the intense neutron flux of a nuclear explosion the production of isotopes may occur through successive neutron induced reactions. The pathway to these isotopes illustrates both the complexity of the problem and the need for high quality nuclear data. The growth and decay of radioactive isotopes can follow a similarly complex network. The Bateman equation will be described and modified to apply to the transmutation of isotopes in a high flux reactor. A alternative model of growth and decay, the GD code, that can be applied to fission products will also be described.

Special features of the inverse-beta-decay reaction proceeding on a proton in a reactor-antineutrino flux

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kopeikin, V. I., E-mail: kopeikin46@yandex.ru; Skorokhvatov, M. D., E-mail: skorokhvatov-md@nrcki.ru

2017-03-15

The evolution of the reactor-antineutrino spectrum and the evolution of the spectrum of positrons from the inverse-beta-decay reaction in the course of reactor operation and after reactor shutdown are considered. The present-day status in determining the initial reactor-antineutrino spectrum on the basis of spectra of beta particles from mixtures of products originating from uranium and plutonium fission is described. A local rise of the experimental spectrum of reactor antineutrinos with respect to the expected spectrum is studied.

A massive pulsar in a compact relativistic binary.

PubMed

Antoniadis, John; Freire, Paulo C C; Wex, Norbert; Tauris, Thomas M; Lynch, Ryan S; van Kerkwijk, Marten H; Kramer, Michael; Bassa, Cees; Dhillon, Vik S; Driebe, Thomas; Hessels, Jason W T; Kaspi, Victoria M; Kondratiev, Vladislav I; Langer, Norbert; Marsh, Thomas R; McLaughlin, Maura A; Pennucci, Timothy T; Ransom, Scott M; Stairs, Ingrid H; van Leeuwen, Joeri; Verbiest, Joris P W; Whelan, David G

2013-04-26

Many physically motivated extensions to general relativity (GR) predict substantial deviations in the properties of spacetime surrounding massive neutron stars. We report the measurement of a 2.01 ± 0.04 solar mass (M⊙) pulsar in a 2.46-hour orbit with a 0.172 ± 0.003 M⊙ white dwarf. The high pulsar mass and the compact orbit make this system a sensitive laboratory of a previously untested strong-field gravity regime. Thus far, the observed orbital decay agrees with GR, supporting its validity even for the extreme conditions present in the system. The resulting constraints on deviations support the use of GR-based templates for ground-based gravitational wave detectors. Additionally, the system strengthens recent constraints on the properties of dense matter and provides insight to binary stellar astrophysics and pulsar recycling.

Effects of surface poisons on the oxidation of binary alloys

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hagan, P.S.; Polizzotti, R.S.; Luckman, G.

1985-10-01

A system of reaction-diffusion equations describing the oxidation of binary alloys in environments containing small amounts of surface poisons is analyzed. These poisons reduce the oxygen flux into the alloy, which causes the alloy to oxidize in two stages.During the initial stage, the oxidation reaction occurs in a stationary boundary layer at the alloy surface. Consequently, a thin zone containing a very high concentration of the metal oxide is created at the alloy surface. During the second stage, the oxidation reaction occurs in a moving boundary layer. This leads to a Stefan problem, which is analyzed by using asymptotic andmore » numerical techniques. By comparing the solutions to those of alloys in unpoisoned environments, it is concluded that surface poisons can lead to the formation of protective external oxide scales in alloys which would not normally form such scales. 11 references.« less

Potential cooling of an accretion-heated neutron star crust in the low-mass X-ray binary 1RXS J180408.9-342058

NASA Astrophysics Data System (ADS)

Parikh, A. S.; Wijnands, R.; Degenaar, N.; Ootes, L. S.; Page, D.; Altamirano, D.; Cackett, E. M.; Deller, A. T.; Gusinskaia, N.; Hessels, J. W. T.; Homan, J.; Linares, M.; Miller, J. M.; Miller-Jones, J. C. A.

2017-04-01

We have monitored the transient neutron star low-mass X-ray binary 1RXS J180408.9-342058 in quiescence after its ˜4.5 month outburst in 2015. The source has been observed using Swift and XMM-Newton. Its X-ray spectra were dominated by a thermal component. The thermal evolution showed a gradual X-ray luminosity decay from ˜18 × 1032 to ˜4 × 1032 (D/5.8 kpc)2 erg s-1 between ˜8 and ˜379 d in quiescence, and the inferred neutron star surface temperature (for an observer at infinity; using a neutron star atmosphere model) decreased from ˜100 to ˜71 eV. This can be interpreted as cooling of an accretion-heated neutron star crust. Modelling the observed temperature curve (using nscool) indicated that the source required ˜1.9 MeV per accreted nucleon of shallow heating in addition to the standard deep crustal heating to explain its thermal evolution. Alternatively, the decay could also be modelled without the presence of deep crustal heating, only having a shallow heat source (again ˜1.9 MeV per accreted nucleon was required). However, the XMM-Newton data statistically required an additional power-law component. This component contributed ˜30 per cent of the total unabsorbed flux in 0.5-10 keV energy range. The physical origin of this component is unknown. One possibility is that it arises from low-level accretion. The presence of this component in the spectrum complicates our cooling crust interpretation because it might indicate that the smooth luminosity and temperature decay curves we observed may not be due to crust cooling but due to some other process.

Evaluation of commercial soybean cultivars for reaction to Phomopsis seed decay

USDA-ARS?s Scientific Manuscript database

Phomopsis seed decay (PSD), caused by Phomopsis longicolla (syn. Diaporthe longicolla), is an economically important soybean disease causing poor seed quality. Planting resistant cultivars is one of the most effective means to control PSD. In this study, 16 commercially available maturity groups IV ...

Experimental study of precisely selected evaporation chains in the decay of excited 25Mg

NASA Astrophysics Data System (ADS)

Camaiani, A.; Casini, G.; Morelli, L.; Barlini, S.; Piantelli, S.; Baiocco, G.; Bini, M.; Bruno, M.; Buccola, A.; Cinausero, M.; Cicerchia, M.; D'Agostino, M.; Degelier, M.; Fabris, D.; Frosin, C.; Gramegna, F.; Gulminelli, F.; Mantovani, G.; Marchi, T.; Olmi, A.; Ottanelli, P.; Pasquali, G.; Pastore, G.; Valdré, S.; Verde, G.

2018-04-01

The reaction 12C+13C at 95 MeV bombarding energy is studied using the Garfield + Ring Counter apparatus located at the INFN Laboratori Nazionali di Legnaro. In this paper we want to investigate the de-excitation of 25Mg aiming both at a new stringent test of the statistical description of nuclear decay and a direct comparison with the decay of the system 24Mg formed through 12C+12C reactions previously studied. Thanks to the large acceptance of the detector and to its good fragment identification capabilities, we could apply stringent selections on fusion-evaporation events, requiring their completeness in charge. The main decay features of the evaporation residues and of the emitted light particles are overall well described by a pure statistical model; however, as for the case of the previously studied 24Mg, we observed some deviations in the branching ratios, in particular for those chains involving only the evaporation of α particles. From this point of view the behavior of the 24Mg and 25Mg decay cases appear to be rather similar. An attempt to obtain a full mass balance even without neutron detection is also discussed.

Tidal disruption of stars in a supermassive black hole binary system: the influence of orbital properties on fallback and accretion rates

NASA Astrophysics Data System (ADS)

Vigneron, Quentin; Lodato, Giuseppe; Guidarelli, Alessio

2018-06-01

The disruption of a star by a supermassive black hole generates a sudden bright flare. Previous studies have focused on the disruption by single black holes, for which the fallback rate decays as ∝ t-5/3. In this paper, we generalize the study to the case of a supermassive black hole binary (SMBHB), using both analytical estimates and hydrodynamical simulations, looking for specific observable signatures. The range of binary separation for which it is possible to distinguish between the disruption created by a single or a binary black hole concerns typically separations of the order of a few milliparsecs for a primary of mass ˜106 M⊙. When the fallback rate is affected by the secondary, it undergoes two types interruptions, depending on the initial inclination θ of the orbit of the star relative to the plane of the SMBHB. For θ ≲ 70°, periodic sharp interruptions occur and the time of first interruption depends on the distance of the secondary black hole with the debris. If θ ≳ 70°, a first smooth interruption occurs, but not always followed by a further recovery of the fallback rate. This implies that most of the TDEs around a SMBHB will undergo periodic sharp interruptions of their light curve.

Measurement of the 169Tm (n ,3 n ) 167Tm cross section and the associated branching ratios in the decay of 167Tm

NASA Astrophysics Data System (ADS)

Champine, B.; Gooden, M. E.; Krishichayan, Norman, E. B.; Scielzo, N. D.; Stoyer, M. A.; Thomas, K. J.; Tonchev, A. P.; Tornow, W.; Wang, B. S.

2016-01-01

The cross section for the 169Tm(n ,3 n ) 167Tm reaction was measured from 17 to 22 MeV using quasimonoenergetic neutrons produced by the 2H(d ,n ) 3He reaction. This energy range was studied to resolve the discrepancy between previous (n ,3 n ) cross-section measurements. In addition, the absolute γ -ray branching ratios following the electron-capture decay of 167Tm were measured. These results provide more reliable nuclear data for an important diagnostic that is used at the National Ignition Facility to estimate the yield of reaction-in-flight neutrons produced via the inertial-confinement-fusion plasma in deuterium-tritium capsules.

Donor-bridge-acceptor energetics determine the distance dependence of electron tunneling in DNA

NASA Astrophysics Data System (ADS)

Lewis, Frederick D.; Liu, Jianqin; Weigel, Wilfried; Rettig, Wolfgang; Kurnikov, Igor V.; Beratan, David N.

2002-10-01

Electron transfer (ET) processes in DNA are of current interest because of their involvement in oxidative strand cleavage reactions and their relevance to the development of molecular electronics. Two mechanisms have been identified for ET in DNA, a single-step tunneling process and a multistep charge-hopping process. The dynamics of tunneling reactions depend on both the distance between the electron donor and acceptor and the nature of the molecular bridge separating the donor and acceptor. In the case of protein and alkane bridges, the distance dependence is not strongly dependent on the properties of the donor and acceptor. In contrast, we show here that the distance decay of DNA ET rates varies markedly with the energetics of the donor and acceptor relative to the bridge. Specifically, we find that an increase in the energy of the bridge states by 0.25 eV (1 eV = 1.602 × 1019 J) relative to the donor and acceptor energies for photochemical oxidation of nucleotides, without changing the reaction free energy, results in an increase in the characteristic exponential distance decay constant for the ET rates from 0.71 to 1.1 Å1. These results show that, in the small tunneling energy gap regime of DNA ET, the distance dependence is not universal; it varies strongly with the tunneling energy gap. These DNA ET reactions fill a "missing link" or transition regime between the large barrier (rapidly decaying) tunneling regime and the (slowly decaying) hopping regime in the general theory of bridge-mediated ET processes.

ATOMIC PHYSICS, AN AUTOINSTRUCTIONAL PROGRAM, VOLUME 3, SUPPLEMENT.

ERIC Educational Resources Information Center

DETERLINE, WILLIAM A.; KLAUS, DAVID J.

THE AUTOINSTRUCTIONAL MATERIALS IN THIS TEXT WERE PREPARED FOR USE IN AN EXPERIMENTAL STUDY, OFFERING SELF-TUTORING MATERIAL FOR LEARNING ATOMIC PHYSICS. THE TOPICS COVERED ARE (1) NUCLEAR BINDING ENERGY, (2) DISCOVERY OF RADIOACTIVITY, (3) RADIOACTIVE RADIATIONS, (4) ALPHA AND BETA DECAY, (5) BETA DECAY REACTIONS, (6) RADIOACTIVE DATING AND…

NNDC Tools and Publications

Science.gov Websites

Site Index NNDC Tools and Publications Nuclear Structure and Decay Tools Nuclear Reaction Tools Nuclear Structure and Decay Tools 2016 Atomic Mass Evaluation Atomic mass evaluation, by Wang, Audi values as a function of gamma energy and multipolarity. Calculations based on I.M. Band and S. Raman

Organometallic Routes into the Nanorealms of Binary Fe-Si Phases

PubMed Central

Kolel-Veetil, Manoj K.; Keller, Teddy M.

2010-01-01

The Fe-Si binary system provides several iron silicides that have varied and exceptional material properties with applications in the electronic industry. The well known Fe-Si binary silicides are Fe3Si, Fe5Si3, FeSi, α-FeSi2 and β-FeSi2. While the iron-rich silicides Fe3Si and Fe5Si3 are known to be room temperature ferromagnets, the stoichiometric FeSi is the only known transition metal Kondo insulator. Furthermore, Fe5Si3 has also been demonstrated to exhibit giant magnetoresistance (GMR). The silicon-rich β-FeSi2 is a direct band gap material usable in light emitting diode (LED) applications. Typically, these silicides are synthesized by traditional solid-state reactions or by ion beam-induced mixing (IBM) of alternating metal and silicon layers. Alternatively, the utilization of organometallic compounds with reactive transition metal (Fe)-carbon bonds has opened various routes for the preparation of these silicides and the silicon-stabilized bcc- and fcc-Fe phases contained in the Fe-Si binary phase diagram. The unique interfacial interactions of carbon with the Fe and Si components have resulted in the preferential formation of nanoscale versions of these materials. This review will discuss such reactions.

Timing and Spectral Study of 4U 1538-52

NASA Technical Reports Server (NTRS)

Clark, George W.

2000-01-01

Improved orbital parameters of the high-mass binary X-ray pulsar 4U 1538-52 have been derived from high count rate data obtained from the Rossi X-Ray Timing Explorer. Pulse-timing analysis yields an eccentricity of 0.174 +/- 0.015, a periastron at 64 deg +/- 9 deg, and evidence of orbital decay with prime-P(sub orb)/P(sub orb) = (-2.9 +/- 2.1) x 10(exp -6)/yr.

Experimental study of the rearrangements of valence protons and neutrons amongst single-particle orbits during double- β decay in Mo 100

DOE PAGES

Freeman, S. J.; Sharp, D. K.; McAllister, S. A.; ...

2017-11-27

The rearrangements of protons and neutrons amongst the valence single-particle orbitals during double-beta decay of Mo-100 have been determined by measuring cross sections in (d, p), (p, d), (He-3, a), and (He-3, d) reactions on Mo-98,Mo-100 and Ru-100,Ru-102 targets. The deduced nucleon occupancies reveal significant discrepancies when compared with theoretical calculations; the same calculations have previously been used to determine the nuclear matrix element associated with the decay probability of double-beta decay of the Mo-100 system.

Measurement of the π 0 → e + e - γ Dalitz decay at the Mainz Microtron

DOE Office of Scientific and Technical Information (OSTI.GOV)

Adlarson, P.; Afzal, F.; Aguar-Bartolomé, P.

The Dalitz decay π 0 → e +e -γ has been measured in the γp → π 0p reaction with the A2 tagged-photon facility at the Mainz Microtron, MAMI. The value obtained for the slope parameter of the π 0 electromagnetic transition form factor, a π= 0.030 ± 0.010 tot, is in agreement with existing measurements of this decay and with recent theoretical calculations. The uncertainty obtained in the value of a π is lower than in previous results based on the π 0 → e +e -γ decay.

Experimental study of the rearrangements of valence protons and neutrons amongst single-particle orbits during double- β decay in Mo 100

DOE Office of Scientific and Technical Information (OSTI.GOV)

Freeman, S. J.; Sharp, D. K.; McAllister, S. A.

The rearrangements of protons and neutrons amongst the valence single-particle orbitals during double-beta decay of Mo-100 have been determined by measuring cross sections in (d, p), (p, d), (He-3, a), and (He-3, d) reactions on Mo-98,Mo-100 and Ru-100,Ru-102 targets. The deduced nucleon occupancies reveal significant discrepancies when compared with theoretical calculations; the same calculations have previously been used to determine the nuclear matrix element associated with the decay probability of double-beta decay of the Mo-100 system.

Experimental study of the rearrangements of valence protons and neutrons amongst single-particle orbits during double-β decay in 100Mo

NASA Astrophysics Data System (ADS)

Freeman, S. J.; Sharp, D. K.; McAllister, S. A.; Kay, B. P.; Deibel, C. M.; Faestermann, T.; Hertenberger, R.; Mitchell, A. J.; Schiffer, J. P.; Szwec, S. V.; Thomas, J. S.; Wirth, H.-F.

2017-11-01

The rearrangements of protons and neutrons amongst the valence single-particle orbitals during double-β decay of 100Mo have been determined by measuring cross sections in (d ,p ), (p ,d ), (3He,α ), and (3He,d ) reactions on Mo,10098 and Ru,102100 targets. The deduced nucleon occupancies reveal significant discrepancies when compared with theoretical calculations; the same calculations have previously been used to determine the nuclear matrix element associated with the decay probability of double-β decay of the 100Mo system.

Measurement of the π 0 → e + e - γ Dalitz decay at the Mainz Microtron

DOE PAGES

Adlarson, P.; Afzal, F.; Aguar-Bartolomé, P.; ...

2017-02-09

The Dalitz decay π 0 → e +e -γ has been measured in the γp → π 0p reaction with the A2 tagged-photon facility at the Mainz Microtron, MAMI. The value obtained for the slope parameter of the π 0 electromagnetic transition form factor, a π= 0.030 ± 0.010 tot, is in agreement with existing measurements of this decay and with recent theoretical calculations. The uncertainty obtained in the value of a π is lower than in previous results based on the π 0 → e +e -γ decay.

Decay property of sup 20 Na for the onset mechanism of the rapid-proton process

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kubono, S.; Ikeda, N.; Funatsu, Y.

1992-07-01

The decay property of {sup 20}Na was studied using a {sup 20}Mg beam to learn better the onset mechanism of the rapid-proton process. The delayed protons were successfully measured, which correspond to one of the possible 1{sup +} states in {sup 20}Na. There is no clear beta decay to the first excited 1{sup +} state above the proton threshold, suggesting that this state would not be the {ital s}-wave resonance in the thermal reaction of {sup 19}Ne+{ital p} as was expected before. The half-life time of {sup 20}Mg is determined to be 114{plus minus}17 ms. The stellar reaction rate ofmore » {sup 19}Ne({ital p},{gamma}){sup 20}Na is also discussed based on the present experimental result.« less

Mechanism of the atmospheric oxidation of sulfur dioxide - Catalysis by hydroxyl radicals

NASA Technical Reports Server (NTRS)

Margitan, J. J.

1984-01-01

A flash photolysis/resonance fluorescence technique was used to investigate the decay of OH due to the reaction OH + SO2 (+M) to HOSO2 (+M). In the presence of small amounts of NO (10 to the 14th per cu cm), the decays deviated from the normal semilogarithmic linearity due to reformation of OH. On the basis of computer simulations of the decay curves, it is suggested that the reactions HOSO2 + O2 to HO2 + SO3 (k3), and HO2 + HO to OH + NO2 are the likely subsequent steps in SO2 oxidation. The upper limit for the binding energy of HOSO2 relative to OH + SO2 is estimated to be 32 kcal/mol. The atmospheric implications of a catalytic oxidation mechanism are briefly discussed.

Nuclear Data Sheets for A = 222

DOE Office of Scientific and Technical Information (OSTI.GOV)

Singh, S.; Tuli, J.; Jain,A.K.

The ENSDF evaluation for A=222 mass chain (1996El01) has been updated on the basis of the experimental results, since September 1995 (literature cutoff date in 1996El01), from various reaction and decay studies for all nuclides in A=222 mass chain (Z=84 to 92). A new nuclide ({sup 222}Po) has since been observed. In addition, new measurements have been reported in Rn, Th and Ra nuclides. The results obtained from various theoretical studies are given as comments. The updated level and decay schemes, and experimental decay and reaction data on which they are based, are summarized and presented for all the nuclidesmore » with mass number A=222. The adopted values of level energies, level spins and parities are given, and {gamma}-ray energies, intensities, as well as other nuclear properties are presented.« less

Measurements of the {sup 116}Cd(p,n) and {sup 116}Sn(n,p) reactions at 300 MeV for studying Gamow-Teller transition strengths in the intermediate nucleus of the {sup 116}Cd double-{beta} decay

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sasano, M.; Kuboki, H.; Sekiguchi, K.

2009-11-09

The double differential cross sections for the {sup 116}Cd(p,n) and {sup 116}Sn(n,p) reactions at 300 MeV have been measured over a wide excitation-energy region including Gamow-Teller (GT) giant resonance (GTGR) for studying GT transition strengths in the intermediate nucleus of the {sup 116}Cd double-{beta} decay, namely {sup 116}In. A large amount of the strengths in the {beta}{sup +} direction has been newly found in the energy region up to 30 MeV, which may imply that the GT strengths in the GTGR region contribute to the nuclear matrix element of the two-neutrino double-{beta} decay.

Price dynamics in political prediction markets

PubMed Central

Majumder, Saikat Ray; Diermeier, Daniel; Rietz, Thomas A.; Amaral, Luís A. Nunes

2009-01-01

Prediction markets, in which contract prices are used to forecast future events, are increasingly applied to various domains ranging from political contests to scientific breakthroughs. However, the dynamics of such markets are not well understood. Here, we study the return dynamics of the oldest, most data-rich prediction markets, the Iowa Electronic Presidential Election “winner-takes-all” markets. As with other financial markets, we find uncorrelated returns, power-law decaying volatility correlations, and, usually, power-law decaying distributions of returns. However, unlike other financial markets, we find conditional diverging volatilities as the contract settlement date approaches. We propose a dynamic binary option model that captures all features of the empirical data and can potentially provide a tool with which one may extract true information events from a price time series. PMID:19155442

Disordered Nuclear Pasta, Magnetic Field Decay, and Crust Cooling in Neutron Stars

NASA Astrophysics Data System (ADS)

Horowitz, C. J.; Berry, D. K.; Briggs, C. M.; Caplan, M. E.; Cumming, A.; Schneider, A. S.

2015-01-01

Nuclear pasta, with nonspherical shapes, is expected near the base of the crust in neutron stars. Large-scale molecular dynamics simulations of pasta show long lived topological defects that could increase electron scattering and reduce both the thermal and electrical conductivities. We model a possible low-conductivity pasta layer by increasing an impurity parameter Qimp . Predictions of light curves for the low-mass x-ray binary MXB 1659-29, assuming a large Qimp, find continued late time cooling that is consistent with Chandra observations. The electrical and thermal conductivities are likely related. Therefore, observations of late time crust cooling can provide insight on the electrical conductivity and the possible decay of neutron star magnetic fields (assuming these are supported by currents in the crust).

Disordered nuclear pasta, magnetic field decay, and crust cooling in neutron stars.

PubMed

Horowitz, C J; Berry, D K; Briggs, C M; Caplan, M E; Cumming, A; Schneider, A S

2015-01-23

Nuclear pasta, with nonspherical shapes, is expected near the base of the crust in neutron stars. Large-scale molecular dynamics simulations of pasta show long lived topological defects that could increase electron scattering and reduce both the thermal and electrical conductivities. We model a possible low-conductivity pasta layer by increasing an impurity parameter Q_{imp}. Predictions of light curves for the low-mass x-ray binary MXB 1659-29, assuming a large Q_{imp}, find continued late time cooling that is consistent with Chandra observations. The electrical and thermal conductivities are likely related. Therefore, observations of late time crust cooling can provide insight on the electrical conductivity and the possible decay of neutron star magnetic fields (assuming these are supported by currents in the crust).

Ionizing radiation-induced destruction of benzene and dienes in aqueous media.

PubMed

Al-Sheikhly, Mohamad; Poster, Dianne L; An, Jung-Chul; Neta, Pedatsur; Silverman, Joseph; Huie, Robert E

2006-05-01

Pulse radiolysis with spectrophotometric and conductometric detection was utilized to study the formation and reactions of radicals from benzene and dienes in aqueous solutions. The benzene OH adduct, *C6H6OH, reacts with O2 (k = 3 x 10(8) L mol(-1) s(-1)) in a reversible reaction. The peroxyl radical, HOC6H6O2*, undergoes O2*- elimination, bimolecular decay, and reaction with benzene to initiate a chain reaction, depending on the dose rate, benzene concentration, and pH. The occurrence of the chain reaction is demonstrated in low-dose-rate gamma radiolysis experiments where the consumption of O2 was monitored. 1,4-Cyclohexadiene, 1,4-hexadiene, and 1,4-pentadiene form OH-adducts and undergo H-abstraction by O*- radicals. The OH-adducts react with O2 to form peroxyl radicals. These peroxyl radicals, however, do not undergo unimolecular O2*- elimination but rather decay by second-order processes, which lead to subsequent steps of O2*- elimination.

Magnetic field decay in black widow pulsars

NASA Astrophysics Data System (ADS)

Mendes, Camile; de Avellar, Marcio G. B.; Horvath, J. E.; Souza, Rodrigo A. de; Benvenuto, O. G.; De Vito, M. A.

2018-04-01

We study in this work the evolution of the magnetic field in `redback-black widow' pulsars. Evolutionary calculations of these `spider' systems suggest that first the accretion operates in the redback stage, and later the companion star ablates matter due to winds from the recycled pulsar. It is generally believed that mass accretion by the pulsar results in a rapid decay of the magnetic field when compared to the rate of an isolated neutron star. We study the evolution of the magnetic field in black widow pulsars by solving numerically the induction equation using the modified Crank-Nicolson method with intermittent episodes of mass accretion on to the neutron star. Our results show that the magnetic field does not fall below a minimum value (`bottom field') in spite of the long evolution time of the black widow systems, extending the previous conclusions for much younger low-mass X-ray binary systems. We find that in this scenario, the magnetic field decay is dominated by the accretion rate, and that the existence of a bottom field is likely related to the fact that the surface temperature of the pulsar does not decay as predicted by the current cooling models. We also observe that the impurity of the pulsar crust is not a dominant factor in the decay of magnetic field for the long evolution time of black widow systems.

Self-assembly of Nano-rods in Photosensitive Phase Separation

NASA Astrophysics Data System (ADS)

Liu, Ya; Kuksenok, Olga; Maresov, Egor; Balazs, Anna

2012-02-01

Computer simulations reveal how photo-induced chemical reactions in polymeric mixtures can be exploited to create long-range order in materials whose features range from the sub-micron to the nanoscale. The process is initiated by shining a spatially uniform light on a photosensitive AB binary blend, which thereby undergoes both a reversible chemical reaction and phase separation. When a well-collimated, higher intensity light is rastered over the sample, the system forms defect-free, spatially periodic structures. We now build on this approach by introducing nanorods that have a preferential affinity for one the phases in a binary mixture. By rastering over the sample with the higher intensity light, we can create ordered arrays of rods within periodically ordered materials in essentially one processing step.

Application of Bogolyubov's theory of weakly nonideal Bose gases to the A+A, A+B, B+B reaction-diffusion system

NASA Astrophysics Data System (ADS)

Konkoli, Zoran

2004-01-01

Theoretical methods for dealing with diffusion-controlled reactions inevitably rely on some kind of approximation, and to find the one that works on a particular problem is not always easy. Here the approximation used by Bogolyubov to study a weakly nonideal Bose gas, referred to as the weakly nonideal Bose gas approximation (WBGA), is applied in the analysis of three reaction-diffusion models: (i) A+A→Ø, (ii) A+B→Ø, and (iii) A+A,B+B,A+B→Ø (the ABBA model). Two types of WBGA are considered, the simpler WBGA-I and the more complicated WBGA-II. All models are defined on the lattice to facilitate comparison with computer experiment (simulation). It is found that the WBGA describes the A+B reaction well, it reproduces the correct d/4 density decay exponent. However, it fails in the case of the A+A reaction and the ABBA model. (To cure the deficiency of WBGA in dealing with the A+A model, a hybrid of the WBGA and Kirkwood superposition approximations is suggested.) It is shown that the WBGA-I is identical to the dressed-tree calculation suggested by Lee [J. Phys. A 27, 2633 (1994)], and that the dressed-tree calculation does not lead to the d/2 density decay exponent when applied to the A+A reaction, as normally believed, but it predicts the d/4 decay exponent. Last, the usage of the small n0 approximation suggested by Mattis and Glasser [Rev. Mod. Phys. 70, 979 (1998)] is questioned if used beyond the A+B reaction-diffusion model.

Spatiotemporal chaos of self-replicating spots in reaction-diffusion systems.

PubMed

Wang, Hongli; Ouyang, Qi

2007-11-23

The statistical properties of self-replicating spots in the reaction-diffusion Gray-Scott model are analyzed. In the chaotic regime of the system, the spots that dominate the spatiotemporal chaos grow and divide in two or decay into the background randomly and continuously. The rates at which the spots are created and decay are observed to be linearly dependent on the number of spots in the system. We derive a probabilistic description of the spot dynamics based on the statistical independence of spots and thus propose a characterization of the spatiotemporal chaos dominated by replicating spots.

Nuclear Data Sheets for A = 196

NASA Astrophysics Data System (ADS)

Xiaolong, Huang

2007-06-01

The 1998 version of nuclear data sheets for A = 196 has been revised and updated on the basis of the experimental results from various decay and reaction studies before January 2006. The experimental data for all known nuclei of A = 196 (Os,Ir,Pt,Au,Hg, Tl,Pb,Bi,Po,At,Rn) have been reevaluated. The experimental methods, references,Jπ arguments,and necessary comments are given in the text. Summary band structure drawings and level schemes from both radioactive decay and reaction studies are presented. Also of special interest are the new identification of superdeformed bands in 196Pb and 196Bi.

A substrate radical intermediate in the reaction between ribonucleotide reductase from Escherichia coli and 2'-azido-2'-deoxynucleoside diphosphates.

PubMed

Sjöberg, B M; Gräslund, A; Eckstein, F

1983-07-10

The B2 subunit of ribonucleotide reductase from Escherichia coli contains a tyrosine radical which is essential for enzyme activity. In the reaction between ribonucleotide reductase and the substrate analogue 2'-azido-2'-deoxycytidine 5'-diphosphate a new transient radical is formed. The EPR characteristics of this new radical species are consistent with a localization of the unpaired electron at the sugar moiety of the nucleotide. The radical shows hyperfine couplings to a hydrogen and a nitrogen nucleus, the latter probably being part of the azide substituent. The formation of the nucleotide radical in this suicidal reaction is concomitant with the decay of the tyrosine radical of the B2 subunit. Kinetic data argue for a first (pseudosecond) order decay of the B2 radical via generation of the nucleotide radical followed by a slower first order decay of the nucleotide radical. End products in the reaction are cytosine and radical-free protein B2. In the reaction between bacteriophage T4 ribonucleotide reductase and 2'-azido-2'-deoxycytidine 5'-diphosphate an identical nucleotide radical is formed. The present results are consistent with the hypothesis that the appearance and structure of the transient radical mimic stages in the normal reaction pathway of ribonucleotide reductase, postulated to proceed via 3'-hydrogen abstraction and cation radical formation of the substrate nucleotide (Stubbe, J., and Ackles, D. (1980) J. Biol. Chem. 255, 8027-8030). The nucleotide radical described here might be equivalent to such a cation radical intermediate.

A kinetic study on sesame cake protein hydrolysis by Alcalase.

PubMed

Demirhan, Elçin; Apar, Dilek Kılıç; Özbek, Belma

2011-01-01

In the present study, the hydrolysis of sesame cake protein was performed by Alcalase, a bacterial protease produced by Bacillus licheniformis, to investigate the reaction kinetics of sesame cake hydrolysis and to determine decay and product inhibition effects for Alcalase. The reactions were carried out for 10 min in 0.1 L of aqueous solutions containing 10, 15, 20, 25, and 30 g protein/L at various temperature and pH values. To determine decay and product inhibition effects for Alcalase, a series of inhibition experiments were conducted with the addition of various amounts of hydrolysate. The reaction kinetics was investigated by initial rate approach. The initial reaction rates were determined from the slopes of the linear models that fitted to the experimental data. The kinetic parameters, K(m) and V(max), were estimated as 41.17 g/L and 9.24 meqv/L x min. The Lineweaver-Burk plots showed that the type of inhibition for Alcalase determined as uncompetitive, and the inhibition constant, K(i), was estimated as 38.24% (hydrolysate/substrate mixture). Practical Application: Plant proteins are increasingly being used as an alternative to proteins from animal sources to perform functional roles in food formulation. Knowledge of the kinetics of the hydrolysis reaction is essential for the optimization of enzymatic protein hydrolysis and for increasing the utilization of plant proteins in food products. Therefore, in the present study, the hydrolysis of sesame cake protein was performed by Alcalase, a bacterial protease produced by B. licheniformis, to investigate the reaction kinetics of sesame cake hydrolysis and to determine decay and product inhibition effects for Alcalase.

Positron-electron decay of 28Si at an excitation energy of 50 MeV

NASA Astrophysics Data System (ADS)

Buda, A.; Bacelar, J. C.; Balanda, A.; van der Ploeg, H.; Sujkowski, Z.; van der Woude, A.

1993-03-01

The electron-position pair decay of 28Si at 50 MeV excitation produced by the isospin T=0 (α + 24Mg) and the mixed isospin T=0,1 (3He + 25Mg) reactions has been studied using a special designed Positron-Electron pair spectrometer PEPSI.

BAYESIAN PARAMETER ESTIMATION IN A MIXED-ORDER MODEL OF BOD DECAY. (U915590)

EPA Science Inventory

We describe a generalized version of the BOD decay model in which the reaction is allowed to assume an order other than one. This is accomplished by making the exponent on BOD concentration a free parameter to be determined by the data. This "mixed-order" model may be ...

Probing the effect of neutron excess on the dynamics of Hf compound system

NASA Astrophysics Data System (ADS)

Sharma, Ishita; Kumar, Raj; Sharma, Manoj K.

2018-05-01

The reaction dynamics of 170Hf* and 174Hf* compound systems formed in 46,50Ti +124Sn reactions have been analyzed within the framework of Dynamical Cluster-decay Model (DCM) over an energy range of Ec.m.=115-156 MeV. The experimental data of fusion evaporation cross sections for 170,174Hf* systems is successfully addressed by optimizing the value of neck length ΔR. It is to be noted that calculations are performed by taking quadrupole deformations β2 with the optimum orientation of decaying fragments. Here, the effect of neutron excess has been examined on the structural properties of decaying fragments via fragmentation potential and preformation probability. The observation depicts that the isotopic effect prevails at fission region and as we move from lighter nucleus i.e. 170Hf* to heavier nucleus i.e. 174Hf*, the heavy mass fragments (HMF) start contributing along with fission fragments which are equally evident for 170Hf* as well. The ΔR values so obtained are compared at center of mass-energies which consequently provides information regarding the relative time scale of decaying fragments.

Evidence of soluble microbial products accelerating chloramine decay in nitrifying bulk water samples.

PubMed

Bal Krishna, K C; Sathasivan, Arumugam; Chandra Sarker, Dipok

2012-09-01

The discovery of a microbially derived soluble product that accelerates chloramine decay is described. Nitrifying bacteria are believed to be wholly responsible for rapid chloramine loss in drinking water systems. However, a recent investigation showed that an unidentified soluble agent significantly accelerated chloramine decay. The agent was suspected to be either natural organic matter (NOM) or soluble microbial products (SMPs). A laboratory scale reactor was fed chloraminated reverse osmosis (RO) treated water to eliminate the interference from NOM. Once nitrification had set in, experiments were conducted on the reactor and feed waters to determine the identity of the component. The study showed the presence of SMPs released by microbes in severely nitrified waters. Further experiments proved that the SMPs significantly accelerated chloramine decay, probably through catalytic reaction. Moreover, application of common protein denaturing techniques stopped the reaction implying that the compound responsible was likely to be a protein. This significant finding will pave the way for better control of chloramine in the distribution systems. Copyright © 2012 Elsevier Ltd. All rights reserved.

Weak decay of hypernuclei

DOE Office of Scientific and Technical Information (OSTI.GOV)

Grace, R.

1983-01-01

The Moby Dick spectrometer (at BNL) in coincidence with a range spectrometer and a TOF neutron detector will be used to study the weak decay modes of /sup 12/C. The Moby Dick spectrometer will be used to reconstruct and tag events in which specific hypernuclear states are formed in the reaction K/sup -/ + /sup 12/C ..-->.. ..pi../sup -/ + /sup 12/C. Subsequent emission of decay products (pions, protons and neutrons) in coincidence with the fast forward pion will be detected in a time and range spectrometer, and a neutron detector.

Volume effects in the decay of free radicals in organic crystals. [cobalt 60 gamma radiation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Markaryan, R.E.; Kovarskii, A.L.; Tshetinin, V.G.

The decay kinetics of the free radicals produced by {gamma}-irradiation of single crystals of organic dicarboxylic acids is studied at hydrostatic pressures up to 200 MPa. Correlation is established between the reaction's activation parameters (V{sup *} and E{sup *}) and the crystals macrocharacteristics - the compressibility and thermal expansion coefficients. A common equation is proposed to describe the variation of the radical decay rate constant with temperature and pressure in malonic, succinic, adipic, glutaric, suberic, and sebacic acids.

Nuclear Data Sheets for A = 52

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dong, Yang; Junde, Huo

2015-09-15

The nuclear structure data belonging to all nuclei with mass number A=52 have been compiled and evaluated using experimental nuclear reaction data and decay data available before July 10, 2015. This evaluaton supersedes the previous publication for this msss chain (2007Hu08, Nuclear Data Sheets 108, 773 (2007)). The data for the ε decay of {sup 52}Co (104 ms) and the ε decay of {sup 52}Ni (40.8 ms) are both incomplete, so new studies would be useful.

Direct measurements of unimolecular and bimolecular reaction kinetics of the Criegee intermediate (CH 3) 2COO

DOE PAGES

Chhantyal-Pun, Rabi; Welz, Oliver; Savee, John D.; ...

2016-10-18

Here, the Criegee intermediate acetone oxide, (CH 3) 2COO, is formed by laser photolysis of 2,2-diiodopropane in the presence of O 2 and characterized by synchrotron photoionization mass spectrometry and by cavity ring-down ultraviolet absorption spectroscopy. The rate coefficient of the reaction of the Criegee intermediate with SO 2 was measured using photoionization mass spectrometry and pseudo-first-order methods to be (7.3 ± 0.5) × 10 –11 cm 3 s –1 at 298 K and 4 Torr and (1.5 ± 0.5) × 10 –10 cm 3 s –1 at 298 K and 10 Torr (He buffer). These values are similar tomore » directly measured rate coefficients of anti-CH 3CHOO with SO 2, and in good agreement with recent UV absorption measurements. The measurement of this reaction at 293 K and slightly higher pressures (between 10 and 100 Torr) in N 2 from cavity ring-down decay of the ultraviolet absorption of (CH 3) 2COO yielded even larger rate coefficients, in the range (1.84 ± 0.12) × 10 –10 to (2.29 ± 0.08) × 10 –10 cm 3 s –1. Photoionization mass spectrometry measurements with deuterated acetone oxide at 4 Torr show an inverse deuterium kinetic isotope effect, kH/kD = (0.53 ± 0.06), for reactions with SO 2, which may be consistent with recent suggestions that the formation of an association complex affects the rate coefficient. The reaction of (CD3)2COO with NO2 has a rate coefficient at 298 K and 4 Torr of (2.1 ± 0.5) × 10 –12 cm 3 s –1 (measured with photoionization mass spectrometry), again similar to rate for the reaction of anti-CH 3CHOO with NO 2. Cavity ring-down measurements of the acetone oxide removal without added reagents display a combination of first- and second-order decay kinetics, which can be deconvolved to derive values for both the self-reaction of (CH 3) 2COO and its unimolecular thermal decay. The inferred unimolecular decay rate coefficient at 293 K, (305 ± 70) s –1, is similar to determinations from ozonolysis. The present measurements confirm the large rate coefficient for reaction of (CH 3) 2COO with SO 2 and the small rate coefficient for its reaction with water. Product measurements of the reactions of (CH 3) 2COO with NO 2 and with SO 2 suggest that these reactions may facilitate isomerization to 2-hydroperoxypropene, possibly by subsequent reactions of association products.« less

Weak decays of heavy hadrons into dynamically generated resonances

DOE PAGES

Oset, Eulogio; Liang, Wei -Hong; Bayar, Melahat; ...

2016-01-28

In this study, we present a review of recent works on weak decay of heavy mesons and baryons with two mesons, or a meson and a baryon, interacting strongly in the final state. The aim is to learn about the interaction of hadrons and how some particular resonances are produced in the reactions. It is shown that these reactions have peculiar features and act as filters for some quantum numbers which allow to identify easily some resonances and learn about their nature. The combination of basic elements of the weak interaction with the framework of the chiral unitary approach allowmore » for an interpretation of results of many reactions and add a novel information to different aspects of the hadron interaction and the properties of dynamically generated resonances.« less

Deriving analytic solutions for compact binary inspirals without recourse to adiabatic approximations

NASA Astrophysics Data System (ADS)

Galley, Chad R.; Rothstein, Ira Z.

2017-05-01

We utilize the dynamical renormalization group formalism to calculate the real space trajectory of a compact binary inspiral for long times via a systematic resummation of secularly growing terms. This method generates closed form solutions without orbit averaging, and the accuracy can be systematically improved. The expansion parameter is v5ν Ω (t -t0) where t0 is the initial time, t is the time elapsed, and Ω and v are the angular orbital frequency and initial speed, respectively. ν is the binary's symmetric mass ratio. We demonstrate how to apply the renormalization group method to resum solutions beyond leading order in two ways. First, we calculate the second-order corrections of the leading radiation reaction force, which involves highly nontrivial checks of the formalism (i.e., its renormalizability). Second, we show how to systematically include post-Newtonian corrections to the radiation reaction force. By avoiding orbit averaging, we gain predictive power and eliminate ambiguities in the initial conditions. Finally, we discuss how this methodology can be used to find analytic solutions to the spin equations of motion that are valid over long times.

Gravitational radiation as a test of relativistic gravity

NASA Technical Reports Server (NTRS)

Will, Clifford M.

1989-01-01

Gravitational radiation can be used to test theories of gravitation. When the waves are ultimately detected directly, their speed and polarization properties can be measured and compared with predictions of alternative theories. The multipole nature of gravitational radiation was already tested in the binary pulsar, where observations of the decay of the orbit verify the quadrupole formula for gravitational radiation damping of general relativity and put strong constraints on dipole gravitational radiation predicted by many alternative theories.

Radio non-detection of Aql X-1

NASA Astrophysics Data System (ADS)

Tudose, V.; Paragi, Z.; Altamirano, D.; Miller-Jones, J. C. A.; Garrett, M.; Fender, R.; Rushton, A.; Spencer, R.; Maitra, D.

2010-10-01

The neutron star X-ray binary Aql X-1 is on the decaying phase of a major outburst that peaked at optical and X-ray bands in mid-September (ATEL #2850, #2871, #2891, #2902). We observed the object at 5 GHz with the European VLBI Network (EVN) in the e-VLBI mode on 2010 October 4th between 18:20-22:09 UT. The participating stations were Cambridge, Effelsberg, Jodrell Bank (MkII), Hartebeesthoek, Medicina, Onsala, Torun, Westerbork and Yebes.

Kilonovae.

PubMed

Metzger, Brian D

2017-01-01

The mergers of double neutron star (NS-NS) and black hole (BH)-NS binaries are promising gravitational wave (GW) sources for Advanced LIGO and future GW detectors. The neutron-rich ejecta from such merger events undergoes rapid neutron capture ( r -process) nucleosynthesis, enriching our Galaxy with rare heavy elements like gold and platinum. The radioactive decay of these unstable nuclei also powers a rapidly evolving, supernova-like transient known as a "kilonova" (also known as "macronova"). Kilonovae are an approximately isotropic electromagnetic counterpart to the GW signal, which also provides a unique and direct probe of an important, if not dominant, r -process site. I review the history and physics of kilonovae, leading to the current paradigm of week-long emission with a spectral peak at near-infrared wavelengths. Using a simple light curve model to illustrate the basic physics, I introduce potentially important variations on this canonical picture, including: [Formula: see text]day-long optical ("blue") emission from lanthanide-free components of the ejecta; [Formula: see text]hour-long precursor UV/blue emission, powered by the decay of free neutrons in the outermost ejecta layers; and enhanced emission due to energy input from a long-lived central engine, such as an accreting BH or millisecond magnetar. I assess the prospects of kilonova detection following future GW detections of NS-NS/BH-NS mergers in light of the recent follow-up campaign of the LIGO binary BH-BH mergers.

Kilonovae

NASA Astrophysics Data System (ADS)

Metzger, Brian D.

2017-05-01

The mergers of double neutron star (NS-NS) and black hole (BH)-NS binaries are promising gravitational wave (GW) sources for Advanced LIGO and future GW detectors. The neutron-rich ejecta from such merger events undergoes rapid neutron capture ( r-process) nucleosynthesis, enriching our Galaxy with rare heavy elements like gold and platinum. The radioactive decay of these unstable nuclei also powers a rapidly evolving, supernova-like transient known as a "kilonova" (also known as "macronova"). Kilonovae are an approximately isotropic electromagnetic counterpart to the GW signal, which also provides a unique and direct probe of an important, if not dominant, r-process site. I review the history and physics of kilonovae, leading to the current paradigm of week-long emission with a spectral peak at near-infrared wavelengths. Using a simple light curve model to illustrate the basic physics, I introduce potentially important variations on this canonical picture, including: ˜ day-long optical ("blue") emission from lanthanide-free components of the ejecta; ˜ hour-long precursor UV/blue emission, powered by the decay of free neutrons in the outermost ejecta layers; and enhanced emission due to energy input from a long-lived central engine, such as an accreting BH or millisecond magnetar. I assess the prospects of kilonova detection following future GW detections of NS-NS/BH-NS mergers in light of the recent follow-up campaign of the LIGO binary BH-BH mergers.

Study of Analytic Statistical Model for Decay of Light and Medium Mass Nuclei in Nuclear Fragmentation

NASA Technical Reports Server (NTRS)

Cucinotta, Francis A.; Wilson, John W.

1996-01-01

The angular momentum independent statistical decay model is often applied using a Monte-Carlo simulation to describe the decay of prefragment nuclei in heavy ion reactions. This paper presents an analytical approach to the decay problem of nuclei with mass number less than 60, which is important for galactic cosmic ray (GCR) studies. This decay problem of nuclei with mass number less than 60 incorporates well-known levels of the lightest nuclei (A less than 11) to improve convergence and accuracy. A sensitivity study of the model level density function is used to determine the impact on mass and charge distributions in nuclear fragmentation. This angular momentum independent statistical decay model also describes the momentum and energy distribution of emitted particles (n, p, d, t, h, and a) from a prefragment nucleus.

Revisiting big-bang nucleosynthesis constraints on long-lived decaying particles

NASA Astrophysics Data System (ADS)

Kawasaki, Masahiro; Kohri, Kazunori; Moroi, Takeo; Takaesu, Yoshitaro

2018-01-01

We study the effects of long-lived massive particles, which decayed during the big-bang nucleosynthesis (BBN) epoch, on the primordial abundance of light elements. Compared to previous studies, (i) the reaction rates of standard BBN reactions are updated, (ii) the most recent observational data on the light element abundance and cosmological parameters are used, (iii) the effects of the interconversion of energetic nucleons at the time of inelastic scattering with background nuclei are considered, and (iv) the effects of the hadronic shower induced by energetic high-energy antinucleons are included. We compare the theoretical predictions on the primordial abundance of light elements with the latest observational constraints, and we derive upper bounds on the relic abundance of the decaying particle as a function of its lifetime. We also apply our analysis to an unstable gravitino, the superpartner of a graviton in supersymmetric theories, and obtain constraints on the reheating temperature after inflation.

Anomalous decay and scattering processes of the meson

NASA Astrophysics Data System (ADS)

Kubis, Bastian; Plenter, Judith

2015-06-01

We amend a recent dispersive analysis of the anomalous decay process by the effects of the tensor meson, the lowest-lying resonance that can contribute in the system. While the net effects on the measured decay spectrum are small, they may be more pronounced for the analogous decay. There are nonnegligible consequences for the transition form factor, which is an important quantity for the hadronic light-by-light scattering contribution to the muon's anomalous magnetic moment. We predict total and differential cross sections, as well as a marked forward-backward asymmetry, for the crossed process , which could be measured in Primakoff reactions in the future.

The r-process nucleosynthesis and related challenges

NASA Astrophysics Data System (ADS)

Goriely, Stephane; Bauswein, Andreas; Janka, Hans-Thomas; Just, Oliver; Pllumbi, Else

2018-01-01

The rapid neutron-capture process, or r-process, is known to be of fundamental importance for explaining the origin of approximately half of the A > 60 stable nuclei observed in nature. Recently, special attention has been paid to neutron star (NS) mergers following the confirmation by hydrodynamic simulations that a non-negligible amount of matter can be ejected and by nucleosynthesis calculations combined with the predicted astrophysical event rate that such a site can account for the majority of r-material in our Galaxy. We show here that the combined contribution of both the dynamical (prompt) ejecta expelled during binary NS or NS-black hole (BH) mergers and the neutrino and viscously driven outflows generated during the post-merger remnant evolution of relic BH-torus systems can lead to the production of r-process elements from mass number A ≳ 90 up to actinides. The corresponding abundance distribution is found to reproduce the solar distribution extremely well. It can also account for the elemental distributions observed in low-metallicity stars. However, major uncertainties still affect our understanding of the composition of the ejected matter. These concern (i) the β-interactions of electron (anti)neutrinos with free neutrons and protons, as well as their inverse reactions, which may affect the neutron-richness of the matter at the early phase of the ejection, and (ii) the nuclear physics of exotic neutron-rich nuclei, including nuclear structure as well as nuclear interaction properties, which impact the calculated abundance distribution. Both aspects are discussed in the light of recent hydrodynamical simulations of NS mergers and microscopic calculations of nuclear decay and reaction probabilities.

Electrostatic screening in classical Coulomb fluids: exponential or power-law decay or both? An investigation into the effect of dispersion interactions

NASA Astrophysics Data System (ADS)

Kjellander, Roland

2006-04-01

It is shown that the nature of the non-electrostatic part of the pair interaction potential in classical Coulomb fluids can have a profound influence on the screening behaviour. Two cases are compared: (i) when the non-electrostatic part equals an arbitrary finite-ranged interaction and (ii) when a dispersion r-6 interaction potential is included. A formal analysis is done in exact statistical mechanics, including an investigation of the bridge function. It is found that the Coulombic r-1 and the dispersion r-6 potentials are coupled in a very intricate manner as regards the screening behaviour. The classical one-component plasma (OCP) is a particularly clear example due to its simplicity and is investigated in detail. When the dispersion r-6 potential is turned on, the screened electrostatic potential from a particle goes from a monotonic exponential decay, exp(-κr)/r, to a power-law decay, r-8, for large r. The pair distribution function acquire, at the same time, an r-10 decay for large r instead of the exponential one. There still remains exponentially decaying contributions to both functions, but these contributions turn oscillatory when the r-6 interaction is switched on. When the Coulomb interaction is turned off but the dispersion r-6 pair potential is kept, the decay of the pair distribution function for large r goes over from the r-10 to an r-6 behaviour, which is the normal one for fluids of electroneutral particles with dispersion interactions. Differences and similarities compared to binary electrolytes are pointed out.

The Next-Generation PCR-Based Quantification Method for Ambient Waters: Digital PCR.

PubMed

Cao, Yiping; Griffith, John F; Weisberg, Stephen B

2016-01-01

Real-time quantitative PCR (qPCR) is increasingly being used for ambient water monitoring, but development of digital polymerase chain reaction (digital PCR) has the potential to further advance the use of molecular techniques in such applications. Digital PCR refines qPCR by partitioning the sample into thousands to millions of miniature reactions that are examined individually for binary endpoint results, with DNA density calculated from the fraction of positives using Poisson statistics. This direct quantification removes the need for standard curves, eliminating the labor and materials associated with creating and running standards with each batch, and removing biases associated with standard variability and mismatching amplification efficiency between standards and samples. Confining reactions and binary endpoint measurements to small partitions also leads to other performance advantages, including reduced susceptibility to inhibition, increased repeatability and reproducibility, and increased capacity to measure multiple targets in one analysis. As such, digital PCR is well suited for ambient water monitoring applications and is particularly advantageous as molecular methods move toward autonomous field application.

The Cu-Li-Sn Phase Diagram: Isopleths, Liquidus Projection and Reaction Scheme

PubMed Central

Flandorfer, Hans

2016-01-01

The Cu-Li-Sn phase diagram was constructed based on XRD and DTA data of 60 different alloy compositions. Eight ternary phases and 14 binary solid phases form 44 invariant ternary reactions, which are illustrated by a Scheil-Schulz reaction scheme and a liquidus projection. Phase equilibria as a function of concentration and temperature are shown along nine isopleths. This report together with an earlier publication of our group provides for the first time comprehensive investigations of phase equilibria and respective phase diagrams. Most of the phase equilibria could be established based on our experimental results. Only in the Li-rich part where many binary and ternary compounds are present estimations had to be done which are all indicated by dashed lines. A stable ternary miscibility gap could be found which was predicted by modelling the liquid ternary phase in a recent work. The phase diagrams are a crucial input for material databases and thermodynamic optimizations regarding new anode materials for high-power Li-ion batteries. PMID:27788175

Searching for Rapid Orbital Decay of WASP-18b

NASA Astrophysics Data System (ADS)

Wilkins, Ashlee N.; Delrez, Laetitia; Barker, Adrian J.; Deming, Drake; Hamilton, Douglas; Gillon, Michael; Jehin, Emmanuel

2017-02-01

The WASP-18 system, with its massive and extremely close-in planet, WASP-18b (M p = 10.3M J , a = 0.02 au, P = 22.6 hr), is one of the best-known exoplanet laboratories to directly measure Q‧, the modified tidal quality factor and proxy for efficiency of tidal dissipation, of the host star. Previous analysis predicted a rapid orbital decay of the planet toward its host star that should be measurable on the timescale of a few years, if the star is as dissipative as is inferred from the circularization of close-in solar-type binary stars. We have compiled published transit and secondary eclipse timing (as observed by WASP, TRAPPIST, and Spitzer) with more recent unpublished light curves (as observed by TRAPPIST and Hubble Space Telescope) with coverage spanning nine years. We find no signature of a rapid decay. We conclude that the absence of rapid orbital decay most likely derives from Q‧ being larger than was inferred from solar-type stars and find that Q‧ ≥ 1 × 106, at 95% confidence; this supports previous work suggesting that F stars, with their convective cores and thin convective envelopes, are significantly less tidally dissipative than solar-type stars, with radiative cores and large convective envelopes.

Searching for Rapid Orbital Decay of WASP-18b

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wilkins, Ashlee N.; Deming, Drake; Hamilton, Douglas

2017-02-20

The WASP-18 system, with its massive and extremely close-in planet, WASP-18b ( M{sub p} = 10.3 M{sub J}, a = 0.02 au, P = 22.6 hr), is one of the best-known exoplanet laboratories to directly measure Q ′, the modified tidal quality factor and proxy for efficiency of tidal dissipation, of the host star. Previous analysis predicted a rapid orbital decay of the planet toward its host star that should be measurable on the timescale of a few years, if the star is as dissipative as is inferred from the circularization of close-in solar-type binary stars. We have compiled publishedmore » transit and secondary eclipse timing (as observed by WASP, TRAPPIST, and Spitzer ) with more recent unpublished light curves (as observed by TRAPPIST and Hubble Space Telescope ) with coverage spanning nine years. We find no signature of a rapid decay. We conclude that the absence of rapid orbital decay most likely derives from Q ′ being larger than was inferred from solar-type stars and find that Q ′ ≥ 1 × 10{sup 6}, at 95% confidence; this supports previous work suggesting that F stars, with their convective cores and thin convective envelopes, are significantly less tidally dissipative than solar-type stars, with radiative cores and large convective envelopes.« less

W and Z boson production in p-Pb collisions at √{s_{NN}}=5.02 TeV

NASA Astrophysics Data System (ADS)

Adam, J.; Adamová, D.; Aggarwal, M. M.; Aglieri Rinella, G.; Agnello, M.; Agrawal, N.; Ahammed, Z.; Ahmad, S.; Ahn, S. U.; Aiola, S.; Akindinov, A.; Alam, S. N.; Albuquerque, D. S. D.; Aleksandrov, D.; Alessandro, B.; Alexandre, D.; Alfaro Molina, R.; Alici, A.; Alkin, A.; Alme, J.; Alt, T.; Altinpinar, S.; Altsybeev, I.; Alves Garcia Prado, C.; An, M.; Andrei, C.; Andrews, H. A.; Andronic, A.; Anguelov, V.; Anson, C.; Antičić, T.; Antinori, F.; Antonioli, P.; Anwar, R.; Aphecetche, L.; Appelshäuser, H.; Arcelli, S.; Arnaldi, R.; Arnold, O. W.; Arsene, I. C.; Arslandok, M.; Audurier, B.; Augustinus, A.; Averbeck, R.; Azmi, M. D.; Badalà, A.; Baek, Y. W.; Bagnasco, S.; Bailhache, R.; Bala, R.; Balasubramanian, S.; Baldisseri, A.; Baral, R. C.; Barbano, A. M.; Barbera, R.; Barile, F.; Barnaföldi, G. G.; Barnby, L. S.; Barret, V.; Bartalini, P.; Barth, K.; Bartke, J.; Bartsch, E.; Basile, M.; Bastid, N.; Basu, S.; Bathen, B.; Batigne, G.; Batista Camejo, A.; Batyunya, B.; Batzing, P. C.; Bearden, I. G.; Beck, H.; Bedda, C.; Behera, N. K.; Belikov, I.; Bellini, F.; Bello Martinez, H.; Bellwied, R.; Beltran, L. G. E.; Belyaev, V.; Bencedi, G.; Beole, S.; Bercuci, A.; Berdnikov, Y.; Berenyi, D.; Bertens, R. A.; Berzano, D.; Betev, L.; Bhasin, A.; Bhat, I. R.; Bhati, A. K.; Bhattacharjee, B.; Bhom, J.; Bianchi, L.; Bianchi, N.; Bianchin, C.; Bielčík, J.; Bielčíková, J.; Bilandzic, A.; Biro, G.; Biswas, R.; Biswas, S.; Bjelogrlic, S.; Blair, J. T.; Blau, D.; Blume, C.; Bock, F.; Bogdanov, A.; Boldizsár, L.; Bombara, M.; Bonora, M.; Book, J.; Borel, H.; Borissov, A.; Borri, M.; Bossù, F.; Botta, E.; Bourjau, C.; Braun-Munzinger, P.; Bregant, M.; Broker, T. A.; Browning, T. A.; Broz, M.; Brucken, E. J.; Bruna, E.; Bruno, G. E.; Budnikov, D.; Buesching, H.; Bufalino, S.; Buhler, P.; Buitron, S. A. I.; Buncic, P.; Busch, O.; Buthelezi, Z.; Butt, J. B.; Buxton, J. T.; Cabala, J.; Caffarri, D.; Caines, H.; Caliva, A.; Calvo Villar, E.; Camerini, P.; Carena, F.; Carena, W.; Carnesecchi, F.; Castillo Castellanos, J.; Castro, A. J.; Casula, E. A. R.; Ceballos Sanchez, C.; Cepila, J.; Cerello, P.; Cerkala, J.; Chang, B.; Chapeland, S.; Chartier, M.; Charvet, J. L.; Chattopadhyay, S.; Chattopadhyay, S.; Chauvin, A.; Chelnokov, V.; Cherney, M.; Cheshkov, C.; Cheynis, B.; Chibante Barroso, V.; Chinellato, D. D.; Cho, S.; Chochula, P.; Choi, K.; Chojnacki, M.; Choudhury, S.; Christakoglou, P.; Christensen, C. H.; Christiansen, P.; Chujo, T.; Chung, S. U.; Cicalo, C.; Cifarelli, L.; Cindolo, F.; Cleymans, J.; Colamaria, F.; Colella, D.; Collu, A.; Colocci, M.; Conesa Balbastre, G.; Conesa del Valle, Z.; Connors, M. E.; Contreras, J. G.; Cormier, T. M.; Corrales Morales, Y.; Cortés Maldonado, I.; Cortese, P.; Cosentino, M. R.; Costa, F.; Crkovská, J.; Crochet, P.; Cruz Albino, R.; Cuautle, E.; Cunqueiro, L.; Dahms, T.; Dainese, A.; Danisch, M. C.; Danu, A.; Das, D.; Das, I.; Das, S.; Dash, A.; Dash, S.; De, S.; De Caro, A.; de Cataldo, G.; de Conti, C.; de Cuveland, J.; De Falco, A.; De Gruttola, D.; De Marco, N.; De Pasquale, S.; De Souza, R. D.; Deisting, A.; Deloff, A.; Deplano, C.; Dhankher, P.; Di Bari, D.; Di Mauro, A.; Di Nezza, P.; Di Ruzza, B.; Diaz Corchero, M. A.; Dietel, T.; Dillenseger, P.; Divià, R.; Djuvsland, Ø.; Dobrin, A.; Domenicis Gimenez, D.; Dönigus, B.; Dordic, O.; Drozhzhova, T.; Dubey, A. K.; Dubla, A.; Ducroux, L.; Duggal, A. K.; Dupieux, P.; Ehlers, R. J.; Elia, D.; Endress, E.; Engel, H.; Epple, E.; Erazmus, B.; Erhardt, F.; Espagnon, B.; Esumi, S.; Eulisse, G.; Eum, J.; Evans, D.; Evdokimov, S.; Eyyubova, G.; Fabbietti, L.; Fabris, D.; Faivre, J.; Fantoni, A.; Fasel, M.; Feldkamp, L.; Feliciello, A.; Feofilov, G.; Ferencei, J.; Fernández Téllez, A.; Ferreiro, E. G.; Ferretti, A.; Festanti, A.; Feuillard, V. J. G.; Figiel, J.; Figueredo, M. A. S.; Filchagin, S.; Finogeev, D.; Fionda, F. M.; Fiore, E. M.; Floris, M.; Foertsch, S.; Foka, P.; Fokin, S.; Fragiacomo, E.; Francescon, A.; Francisco, A.; Frankenfeld, U.; Fronze, G. G.; Fuchs, U.; Furget, C.; Furs, A.; Fusco Girard, M.; Gaardhøje, J. J.; Gagliardi, M.; Gago, A. M.; Gajdosova, K.; Gallio, M.; Galvan, C. D.; Gangadharan, D. R.; Ganoti, P.; Gao, C.; Garabatos, C.; Garcia-Solis, E.; Garg, K.; Garg, P.; Gargiulo, C.; Gasik, P.; Gauger, E. F.; Gay Ducati, M. B.; Germain, M.; Ghosh, P.; Ghosh, S. K.; Gianotti, P.; Giubellino, P.; Giubilato, P.; Gladysz-Dziadus, E.; Glässel, P.; Goméz Coral, D. M.; Gomez Ramirez, A.; Gonzalez, A. S.; Gonzalez, V.; González-Zamora, P.; Gorbunov, S.; Görlich, L.; Gotovac, S.; Grabski, V.; Graczykowski, L. K.; Graham, K. L.; Greiner, L.; Grelli, A.; Grigoras, C.; Grigoriev, V.; Grigoryan, A.; Grigoryan, S.; Grion, N.; Gronefeld, J. M.; Grosse-Oetringhaus, J. F.; Grosso, R.; Gruber, L.; Guber, F.; Guernane, R.; Guerzoni, B.; Gulbrandsen, K.; Gunji, T.; Gupta, A.; Gupta, R.; Guzman, I. B.; Haake, R.; Hadjidakis, C.; Hamagaki, H.; Hamar, G.; Hamon, J. C.; Harris, J. W.; Harton, A.; Hatzifotiadou, D.; Hayashi, S.; Heckel, S. T.; Hellbär, E.; Helstrup, H.; Herghelegiu, A.; Herrera Corral, G.; Herrmann, F.; Hess, B. A.; Hetland, K. F.; Hillemanns, H.; Hippolyte, B.; Hladky, J.; Horak, D.; Hosokawa, R.; Hristov, P.; Hughes, C.; Humanic, T. J.; Hussain, N.; Hussain, T.; Hutter, D.; Hwang, D. S.; Ilkaev, R.; Inaba, M.; Ippolitov, M.; Irfan, M.; Isakov, V.; Islam, M. S.; Ivanov, M.; Ivanov, V.; Izucheev, V.; Jacak, B.; Jacazio, N.; Jacobs, P. M.; Jadhav, M. B.; Jadlovska, S.; Jadlovsky, J.; Jahnke, C.; Jakubowska, M. J.; Janik, M. A.; Jayarathna, P. H. S. Y.; Jena, C.; Jena, S.; Jimenez Bustamante, R. T.; Jones, P. G.; Jusko, A.; Kalinak, P.; Kalweit, A.; Kang, J. H.; Kaplin, V.; Kar, S.; Karasu Uysal, A.; Karavichev, O.; Karavicheva, T.; Karayan, L.; Karpechev, E.; Kebschull, U.; Keidel, R.; Keijdener, D. L. D.; Keil, M.; Mohisin Khan, M.; Khan, P.; Khan, S. A.; Khanzadeev, A.; Kharlov, Y.; Khatun, A.; Khuntia, A.; Kileng, B.; Kim, D. W.; Kim, D. J.; Kim, D.; Kim, H.; Kim, J. S.; Kim, J.; Kim, M.; Kim, M.; Kim, S.; Kim, T.; Kirsch, S.; Kisel, I.; Kiselev, S.; Kisiel, A.; Kiss, G.; Klay, J. L.; Klein, C.; Klein, J.; Klein-Bösing, C.; Klewin, S.; Kluge, A.; Knichel, M. L.; Knospe, A. G.; Kobdaj, C.; Kofarago, M.; Kollegger, T.; Kolojvari, A.; Kondratiev, V.; Kondratyeva, N.; Kondratyuk, E.; Konevskikh, A.; Kopcik, M.; Kour, M.; Kouzinopoulos, C.; Kovalenko, O.; Kovalenko, V.; Kowalski, M.; Koyithatta Meethaleveedu, G.; Králik, I.; Kravčáková, A.; Krivda, M.; Krizek, F.; Kryshen, E.; Krzewicki, M.; Kubera, A. M.; Kučera, V.; Kuhn, C.; Kuijer, P. G.; Kumar, A.; Kumar, J.; Kumar, L.; Kumar, S.; Kundu, S.; Kurashvili, P.; Kurepin, A.; Kurepin, A. B.; Kuryakin, A.; Kushpil, S.; Kweon, M. J.; Kwon, Y.; La Pointe, S. L.; La Rocca, P.; Lagana Fernandes, C.; Lakomov, I.; Langoy, R.; Lapidus, K.; Lara, C.; Lardeux, A.; Lattuca, A.; Laudi, E.; Lazaridis, L.; Lea, R.; Leardini, L.; Lee, S.; Lehas, F.; Lehner, S.; Lehrbach, J.; Lemmon, R. C.; Lenti, V.; Leogrande, E.; León Monzón, I.; Lévai, P.; Li, S.; Li, X.; Lien, J.; Lietava, R.; Lindal, S.; Lindenstruth, V.; Lippmann, C.; Lisa, M. A.; Ljunggren, H. M.; Llope, W.; Lodato, D. F.; Loenne, P. I.; Loginov, V.; Loizides, C.; Lopez, X.; López Torres, E.; Lowe, A.; Luettig, P.; Lunardon, M.; Luparello, G.; Lupi, M.; Lutz, T. H.; Maevskaya, A.; Mager, M.; Mahajan, S.; Mahmood, S. M.; Maire, A.; Majka, R. D.; Malaev, M.; Maldonado Cervantes, I.; Malinina, L.; Mal'Kevich, D.; Malzacher, P.; Mamonov, A.; Manko, V.; Manso, F.; Manzari, V.; Mao, Y.; Marchisone, M.; Mareš, J.; Margagliotti, G. V.; Margotti, A.; Margutti, J.; Marín, A.; Markert, C.; Marquard, M.; Martin, N. A.; Martinengo, P.; Martínez, M. I.; Martínez García, G.; Martinez Pedreira, M.; Mas, A.; Masciocchi, S.; Masera, M.; Masoni, A.; Mastroserio, A.; Mathis, A. M.; Matyja, A.; Mayer, C.; Mazer, J.; Mazzilli, M.; Mazzoni, M. A.; Meddi, F.; Melikyan, Y.; Menchaca-Rocha, A.; Meninno, E.; Mercado Pérez, J.; Meres, M.; Mhlanga, S.; Miake, Y.; Mieskolainen, M. M.; Mikhaylov, K.; Milano, L.; Milosevic, J.; Mischke, A.; Mishra, A. N.; Mishra, T.; Miskowiec, D.; Mitra, J.; Mitu, C. M.; Mohammadi, N.; Mohanty, B.; Molnar, L.; Montes, E.; Moreira De Godoy, D. A.; Moreno, L. A. P.; Moretto, S.; Morreale, A.; Morsch, A.; Muccifora, V.; Mudnic, E.; Mühlheim, D.; Muhuri, S.; Mukherjee, M.; Mulligan, J. D.; Munhoz, M. G.; Münning, K.; Munzer, R. H.; Murakami, H.; Murray, S.; Musa, L.; Musinsky, J.; Myers, C. J.; Naik, B.; Nair, R.; Nandi, B. K.; Nania, R.; Nappi, E.; Naru, M. U.; Natal da Luz, H.; Nattrass, C.; Navarro, S. R.; Nayak, K.; Nayak, R.; Nayak, T. K.; Nazarenko, S.; Nedosekin, A.; Negrao De Oliveira, R. A.; Nellen, L.; Ng, F.; Nicassio, M.; Niculescu, M.; Niedziela, J.; Nielsen, B. S.; Nikolaev, S.; Nikulin, S.; Nikulin, V.; Noferini, F.; Nomokonov, P.; Nooren, G.; Noris, J. C. C.; Norman, J.; Nyanin, A.; Nystrand, J.; Oeschler, H.; Oh, S.; Ohlson, A.; Okubo, T.; Olah, L.; Oleniacz, J.; Oliveira Da Silva, A. C.; Oliver, M. H.; Onderwaater, J.; Oppedisano, C.; Orava, R.; Oravec, M.; Ortiz Velasquez, A.; Oskarsson, A.; Otwinowski, J.; Oyama, K.; Ozdemir, M.; Pachmayer, Y.; Pacik, V.; Pagano, D.; Pagano, P.; Paić, G.; Pal, S. K.; Palni, P.; Pan, J.; Pandey, A. K.; Papikyan, V.; Pappalardo, G. S.; Pareek, P.; Park, J.; Park, W. J.; Parmar, S.; Passfeld, A.; Paticchio, V.; Patra, R. N.; Paul, B.; Pei, H.; Peitzmann, T.; Peng, X.; Pereira Da Costa, H.; Peresunko, D.; Perez Lezama, E.; Peskov, V.; Pestov, Y.; Petráček, V.; Petrov, V.; Petrovici, M.; Petta, C.; Piano, S.; Pikna, M.; Pillot, P.; Pimentel, L. O. D. L.; Pinazza, O.; Pinsky, L.; Piyarathna, D. B.; Ploskon, M.; Planinic, M.; Pluta, J.; Pochybova, S.; Podesta-Lerma, P. L. M.; Poghosyan, M. G.; Polichtchouk, B.; Poljak, N.; Poonsawat, W.; Pop, A.; Poppenborg, H.; Porteboeuf-Houssais, S.; Porter, J.; Pospisil, J.; Pozdniakov, V.; Prasad, S. K.; Preghenella, R.; Prino, F.; Pruneau, C. A.; Pshenichnov, I.; Puccio, M.; Puddu, G.; Pujahari, P.; Punin, V.; Putschke, J.; Qvigstad, H.; Rachevski, A.; Raha, S.; Rajput, S.; Rak, J.; Rakotozafindrabe, A.; Ramello, L.; Rami, F.; Rana, D. B.; Raniwala, R.; Raniwala, S.; Räsänen, S. S.; Rascanu, B. T.; Rathee, D.; Ratza, V.; Ravasenga, I.; Read, K. F.; Redlich, K.; Rehman, A.; Reichelt, P.; Reidt, F.; Ren, X.; Renfordt, R.; Reolon, A. R.; Reshetin, A.; Reygers, K.; Riabov, V.; Ricci, R. A.; Richert, T.; Richter, M.; Riedler, P.; Riegler, W.; Riggi, F.; Ristea, C.; Rodríguez Cahuantzi, M.; Røed, K.; Rogochaya, E.; Rohr, D.; Röhrich, D.; Ronchetti, F.; Ronflette, L.; Rosnet, P.; Rossi, A.; Roukoutakis, F.; Roy, A.; Roy, C.; Roy, P.; Rubio Montero, A. J.; Rui, R.; Russo, R.; Ryabinkin, E.; Ryabov, Y.; Rybicki, A.; Saarinen, S.; Sadhu, S.; Sadovsky, S.; Šafařík, K.; Sahlmuller, B.; Sahoo, B.; Sahoo, P.; Sahoo, R.; Sahoo, S.; Sahu, P. K.; Saini, J.; Sakai, S.; Saleh, M. A.; Salzwedel, J.; Sambyal, S.; Samsonov, V.; Sandoval, A.; Sano, M.; Sarkar, D.; Sarkar, N.; Sarma, P.; Sas, M. H. P.; Scapparone, E.; Scarlassara, F.; Scharenberg, R. P.; Schiaua, C.; Schicker, R.; Schmidt, C.; Schmidt, H. R.; Schmidt, M.; Schukraft, J.; Schutz, Y.; Schwarz, K.; Schweda, K.; Scioli, G.; Scomparin, E.; Scott, R.; Šefčík, M.; Seger, J. E.; Sekiguchi, Y.; Sekihata, D.; Selyuzhenkov, I.; Senosi, K.; Senyukov, S.; Serradilla, E.; Sett, P.; Sevcenco, A.; Shabanov, A.; Shabetai, A.; Shadura, O.; Shahoyan, R.; Shangaraev, A.; Sharma, A.; Sharma, A.; Sharma, M.; Sharma, M.; Sharma, N.; Sheikh, A. I.; Shigaki, K.; Shou, Q.; Shtejer, K.; Sibiriak, Y.; Siddhanta, S.; Sielewicz, K. M.; Siemiarczuk, T.; Silvermyr, D.; Silvestre, C.; Simatovic, G.; Simonetti, G.; Singaraju, R.; Singh, R.; Singhal, V.; Sinha, T.; Sitar, B.; Sitta, M.; Skaali, T. B.; Slupecki, M.; Smirnov, N.; Snellings, R. J. M.; Snellman, T. W.; Song, J.; Song, M.; Song, Z.; Soramel, F.; Sorensen, S.; Sozzi, F.; Spiriti, E.; Sputowska, I.; Srivastava, B. K.; Stachel, J.; Stan, I.; Stankus, P.; Stenlund, E.; Steyn, G.; Stiller, J. H.; Stocco, D.; Strmen, P.; Suaide, A. A. P.; Sugitate, T.; Suire, C.; Suleymanov, M.; Suljic, M.; Sultanov, R.; Šumbera, M.; Sumowidagdo, S.; Suzuki, K.; Swain, S.; Szabo, A.; Szarka, I.; Szczepankiewicz, A.; Szymanski, M.; Tabassam, U.; Takahashi, J.; Tambave, G. J.; Tanaka, N.; Tarhini, M.; Tariq, M.; Tarzila, M. G.; Tauro, A.; Tejeda Muñoz, G.; Telesca, A.; Terasaki, K.; Terrevoli, C.; Teyssier, B.; Thakur, D.; Thomas, D.; Tieulent, R.; Tikhonov, A.; Timmins, A. R.; Toia, A.; Tripathy, S.; Trogolo, S.; Trombetta, G.; Trubnikov, V.; Trzaska, W. H.; Tsuji, T.; Tumkin, A.; Turrisi, R.; Tveter, T. S.; Ullaland, K.; Umaka, E. N.; Uras, A.; Usai, G. L.; Utrobicic, A.; Vala, M.; Van Der Maarel, J.; Van Hoorne, J. W.; van Leeuwen, M.; Vanat, T.; Vande Vyvre, P.; Varga, D.; Vargas, A.; Vargyas, M.; Varma, R.; Vasileiou, M.; Vasiliev, A.; Vauthier, A.; Vázquez Doce, O.; Vechernin, V.; Veen, A. M.; Velure, A.; Vercellin, E.; Vergara Limón, S.; Vernet, R.; Vértesi, R.; Vickovic, L.; Vigolo, S.; Viinikainen, J.; Vilakazi, Z.; Villalobos Baillie, O.; Villatoro Tello, A.; Vinogradov, A.; Vinogradov, L.; Virgili, T.; Vislavicius, V.; Vodopyanov, A.; Völkl, M. A.; Voloshin, K.; Voloshin, S. A.; Volpe, G.; von Haller, B.; Vorobyev, I.; Voscek, D.; Vranic, D.; Vrláková, J.; Wagner, B.; Wagner, J.; Wang, H.; Wang, M.; Watanabe, D.; Watanabe, Y.; Weber, M.; Weber, S. G.; Weiser, D. F.; Wessels, J. P.; Westerhoff, U.; Whitehead, A. M.; Wiechula, J.; Wikne, J.; Wilk, G.; Wilkinson, J.; Willems, G. A.; Williams, M. C. S.; Windelband, B.; Winn, M.; Witt, W. E.; Yalcin, S.; Yang, P.; Yano, S.; Yin, Z.; Yokoyama, H.; Yoo, I.-K.; Yoon, J. H.; Yurchenko, V.; Zaccolo, V.; Zaman, A.; Zampolli, C.; Zanoli, H. J. C.; Zaporozhets, S.; Zardoshti, N.; Zarochentsev, A.; Závada, P.; Zaviyalov, N.; Zbroszczyk, H.; Zhalov, M.; Zhang, H.; Zhang, X.; Zhang, Y.; Zhang, C.; Zhang, Z.; Zhao, C.; Zhigareva, N.; Zhou, D.; Zhou, Y.; Zhou, Z.; Zhu, H.; Zhu, J.; Zichichi, A.; Zimmermann, A.; Zimmermann, M. B.; Zinovjev, G.; Zmeskal, J.

2017-02-01

The W and Z boson production was measured via the muonic decay channel in proton-lead collisions at √{s_{NN}}=5.02 TeV at the Large Hadron Collider with the ALICE detector. The measurement covers backward (-4.46 < y cms < -2.96) and forward (2.03 < y cms < 3.53) rapidity regions, corresponding to Pb-going and p-going directions, respectively. The Z-boson production cross section, with dimuon invariant mass of 60 < m μμ < 120 GeV/ c 2 and muon transverse momentum ( p T μ ) larger than 20 GeV/ c, is measured. The production cross section and charge asymmetry of muons from W-boson decays with p T μ > 10 GeV/ c are determined. The results are compared to theoretical calculations both with and without including the nuclear modification of the parton distribution functions. The W-boson production is also studied as a function of the collision centrality: the cross section of muons from W-boson decays is found to scale with the average number of binary nucleon-nucleon collisions within uncertainties.

Reaction of maturity group III soybean plant introductions to Phomopsis seed decay in Arkansas Mississippi and Missouri 2009

USDA-ARS?s Scientific Manuscript database

Soybean Phomopsis seed decay (PSD) is the major cause of poor seed quality in the United States, especially in the mid-south region. The disease is primarily caused by Phomopsis longicolla along with other Phomopsis and Diaporthe spp. There are few management strategies for this disease, and these s...

Reaction of maturity group IV soybean plant introductions to Phomopsis Seed Decay in Arkansas Mississippi and Missouri 2009

USDA-ARS?s Scientific Manuscript database

Soybean Phomopsis seed decay (PSD) causes poor seed quality and suppresses yield in most of soybean-growing states in United States. In 2009, PSD caused over 12 million bushel yield loss in 16 southern states. The disease is primarily caused by Phomopsis longicolla along with other Phomopsis and Dia...

Gene expression analysis of wood decay fungus Fibroporia Radiculosa grown In ACQ-treated wood

Treesearch

Ayfer Akgul; Ali Akgul; Juliet D. Diehl Tang

2018-01-01

Copper-tolerant brown-rot fungi are able todegrade wood treated with copper or copper-based wood preservatives. This research used quantitative reverse transcriptase polymerase chain reaction to explore what genes of the brown-rot fungus, Fibroporia radiculosa, were expressed when the fungus was overcoming the wood preservatives and decaying the...

Nuclear Data Sheets for A = 168

DOE Office of Scientific and Technical Information (OSTI.GOV)

Baglin, Coral M.

2010-07-15

Nuclear structure data pertaining to all nuclei with mass A=168 (Tb, Dy, Ho, Er, Tm, Yb, Lu, Hf, Ta, W, Re, Os, Ir, Pt) have been evaluated and incorporated into the ENSDF data file. This evaluation supersedes the previous publication (V.S. Shirley, Nuclear Data Sheets 71, 261 (1994) (literature cutoff date July 1993)) and subsequent ENSDF file revisions for Tb and Dy (C. Baglin, literature cutoff date of 15 June 1999) and Hf (B. Singh, literature cutoff date of 30 April 2001), and includes literature available by 15 June 2010. Since the above evaluations, the first excited states in {supmore » 168}Pt have been identified (1998Ki20, 2009Go16) and {alpha} decay from {sup 172}Hg has been observed (2009Sa27, 2004Ke06, 1999Se14). New levels in {sup 168}Dy have been excited using the {sup 170}Er({sup 82}Se,{sup 84}Kr{gamma}) reaction (2010So03). (HI,xn{gamma}) studies have significantly expanded our knowledge of level structure in {sup 168}Lu (1999Ka17, 2002Ha33), {sup 168}Ta (2008QiZZ), {sup 168}Yb (1995Fi01), {sup 168}Tm (2007CaZW), {sup 168}Hf (2009Ya21), {sup 168}Os (2001Jo11, 2009Od02) and, for {sup 168}Tm, important information has come also from (d,2n{gamma}) and ({alpha},n{gamma}) reactions (1995Si20). Revised decay schemes are available following new studies of {sup 168}Hf {epsilon} decay (6.7 min) (1997Ba26), {sup 168}Lu {epsilon} decay (1999Ba65), {sup 168}Ta {epsilon} decay (2007Mc08) and {sup 172}Au {alpha} decay (2009Ha42). Significant new information for {sup 168}Er is available from (p,t) (2006Bu09), (d,p) and (t,d) (1996Ma50), ({gamma},{gamma}') (1996Ma18), (136Xe, X{gamma}) (2010Dr02), ({sup 238}U,{sup 238}U{sup '{gamma}}) (2003Wu07) and (n,n{sup '{gamma}}) (1998Be20, 1998Be62) reactions, and the availability of {gamma}{gamma} coin data (1994Ju02, 1996Gi09) for the (n,{gamma}) E=thermal reaction has resulted in some significant level scheme revisions.« less

Mechanism of atomic layer deposition of SiO2 on the silicon (100)-2×1 surface using SiCl4 and H2O as precursors

NASA Astrophysics Data System (ADS)

Kang, Jeung Ku; Musgrave, Charles B.

2002-03-01

We use density functional theory to investigate atomic layer deposition (ALD) mechanism of silicon dioxide on the Si(100)-2×1 surface from the precursors SiCl4 and H2O. First, we explore the reaction mechanism of water with the bare Si(100)-2×1 surface to produce surface hydroxyl groups. We find that this reaction proceeds through a two-step pathway with an overall barrier of 33.3 kcal/mol. Next, we investigate the ALD mechanism for the binary reaction sequence: the SiCl4 half reaction and the H2O half reaction. For the SiCl4 half reaction, SiCl4 first forms a σ-bond with the oxygen of the surface OH group and then releases an HCl molecule. The predicted barrier for this process is 15.8 kcal/mol. Next, adsorbed SiCl3 reacts with a neighboring OH group to form bridged SiCl2 with a barrier of 22.6 kcal/mol. The H2O half reaction also proceeds through two sequential steps with an overall barrier of 19.1 kcal/mol for the reaction of H2O with bridged SiCl2 to form bridged Si(OH)2. The predicted barrier of 22.6 kcal/mol for the rate-limiting step of the ALD binary reaction mechanism is consistent with the experimental value of 22.0 kcal/mol. In addition, we find that the calculated frequencies are in good agreement with the experimentally measured IR spectra.

Relation between proton and neutron asymptotic normalization coefficients for light mirror nuclei and its relevance to nuclear astrophysics.

PubMed

Timofeyuk, N K; Johnson, R C; Mukhamedzhanov, A M

2003-12-05

We show how the charge symmetry of strong interactions can be used to relate the proton and neutron asymptotic normalization coefficients (ANCs) of the one-nucleon overlap integrals for light mirror nuclei. This relation extends to the case of real proton decay where the mirror analog is a virtual neutron decay of a loosely bound state. In this case, a link is obtained between the proton width and the squared ANC of the mirror neutron state. The relation between mirror overlaps can be used to study astrophysically relevant proton capture reactions based on information obtained from transfer reactions with stable beams.

Intermediate Nuclear Structure for 2v 2{beta} Decay of {sup 48}Ca Studied by (p, n) and (n, p) Reactions at 300 MeV

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sakai, H.; Yako, K.

2009-08-26

Angular distributions of the double differential cross sections for the {sup 48}Ca(p,n) and the {sup 48}Ti(n,p) reactions were measured at 300 MeV. A multipole decomposition technique was applied to the spectra to extract the Gamow-Teller (GT) transition strengths. In the (n, p) spectrum beyond 8 MeV excitation energy extra B(GT{sup +}) strengths which are not predicted by the shell model calculation. This extra B(GT{sup +}) strengths significantly contribute to the nuclear matrix element of the 2v2{beta}-decay.

History of Weak Interactions

DOE R&D Accomplishments Database

Lee, T. D.

1970-07-01

While the phenomenon of beta-decay was discovered near the end of the last century, the notion that the weak interaction forms a separate field of physical forces evolved rather gradually. This became clear only after the experimental discoveries of other weak reactions such as muon-decay, muon-capture, etc., and the theoretical observation that all these reactions can be described by approximately the same coupling constant, thus giving rise to the notion of a universal weak interaction. Only then did one slowly recognize that the weak interaction force forms an independent field, perhaps on the same footing as the gravitational force, the electromagnetic force, and the strong nuclear and sub-nuclear forces.

Transient species in the pulse radiolysis of methylene chloride and the self-reaction of chloromethyl radicals

NASA Astrophysics Data System (ADS)

Emmi, S. S.; Beggiato, G.; Casalbore-Miceli, G.

Chlorine atoms formed during the pulse radiolysis of deaerated methylene chloride at room temperature react with the solvent in the first 70 ns from the pulse at a bimolecular rate constant k4 ≈ 6 × 10 6 M -1s -1 and are available to otther reactions only at solute concentrations higher than 10 -3M. A u.v.-vis. spectrum is detected, the main features of which are a peak at 350 nm, a broad absorption in the vis. and a remarkable band in the u.v. The "350" species undertakes a fast first order decay ( k = 9.0 × 10 7s -1) which is followed by a slower decay ( k = 5.3 × 10 4s -1). The "u.v." species is a mixing of mono-and dichloromethyl radicals. These radicals recombine and cross-combine as if they were a single species; a rate constant 2 k 9 = 2 k 10 less than 2.4 × 10 9M -1s -1 for the combination reactions can be evaluated from the observed decay rate. Configurational factors are considered in connection with the reactivity of chlorosubstituted methyl radicals.

The Effectiveness of Al-Si Coatings for Preventing Interfacial Reaction in Al-Mg Dissimilar Metal Welding

NASA Astrophysics Data System (ADS)

Wang, Yin; Al-Zubaidy, Basem; Prangnell, Philip B.

2018-01-01

The dissimilar welding of aluminum to magnesium is challenging because of the rapid formation of brittle intermetallic compounds (IMC) at the weld interface. An Al-Si coating interlayer was selected to address this problem, based on thermodynamic calculations which predicted that silicon would change the reaction path to avoid formation of the normally observed binary Al-Mg IMC phases ( β-Al3Mg2 and γ-Al12Mg17). Long-term static heat treatments confirmed that a Si-rich coating will preferentially produce the Mg2Si phase in competition with the less stable, β-Al3Mg2 and γ-Al12Mg17 binary IMC phases, and this reduced the overall reaction layer thickness. However, when an Al-Si clad sheet was tested in a real welding scenario, using the Refill™ friction stir spot welding (FSSW) technique, Mg2Si was only produced in very small amounts owing to the much shorter reaction time. Surprisingly, the coating still led to a significant reduction in the IMC reaction layer thickness and the welds exhibited enhanced mechanical performance, with improved strength and fracture energy. This beneficial behavior has been attributed to the softer coating material both reducing the welding temperature and giving rise to the incorporation of Si particles into the reaction layer, which toughened the brittle interfacial IMC phases during crack propagation.

Less haste, less waste: on recycling and its limits in strand displacement systems

PubMed Central

Condon, Anne; Hu, Alan J.; Maňuch, Ján; Thachuk, Chris

2012-01-01

We study the potential for molecule recycling in chemical reaction systems and their DNA strand displacement realizations. Recycling happens when a product of one reaction is a reactant in a later reaction. Recycling has the benefits of reducing consumption, or waste, of molecules and of avoiding fuel depletion. We present a binary counter that recycles molecules efficiently while incurring just a moderate slowdown compared with alternative counters that do not recycle strands. This counter is an n-bit binary reflecting Gray code counter that advances through 2n states. In the strand displacement realization of this counter, the waste—total number of nucleotides of the DNA strands consumed—is polynomial in n, the number of bits of the counter, while the waste of alternative counters grows exponentially in n. We also show that our n-bit counter fails to work correctly when many (Θ(n)) copies of the species that represent the bits of the counter are present initially. The proof applies more generally to show that in chemical reaction systems where all but one reactant of each reaction are catalysts, computations longer than a polynomial function of the size of the system are not possible when there are polynomially many copies of the system present. PMID:22649584

A Competitive Kinetics Study of the Reaction of Cl with CS2 in Air at 298 K

NASA Technical Reports Server (NTRS)

Wallington, Timothy J.; Andino, Jean M.; Potts, Alan R.; Wine, Paul H.

1997-01-01

The relative rate technique has been used to investigate the kinetics of the reaction of Cl atoms with carbon disulfide, CS2, at 700 Torr total pressure of air at 298 K. The decay rate of CS2 was measured relative to CH4, CH3Cl and CHF2CL. For experiments using CH4 and CH3Cl references, the decay rate of CS2 was dependent on the ratio of the concentration of the reference to that of CS2. We ascribe this behavior to the generation of OH radicals in the system leading to complicated secondary chemistry. From experiments using CHF2Cl we are able to assign an upper limit of 4 x 10(exp -15) cu cm/(molecule s) for the overall reaction, Cl + CS2 yields products.

Seasonal variation of meteor decay times observed at King Sejong Station (62.22°S, 58.78°W), Antarctica

NASA Astrophysics Data System (ADS)

Kim, Jeong-Han; Kim, Yong Ha; Lee, Chang-Sup; Jee, Geonhwa

2010-07-01

We analyzed meteor decay times measured by a VHF radar at King Sejong Station by classifying strong and weak meteors according to their estimated electron line densities. The height profiles of monthly averaged decay times show a peak whose altitude varies with season at altitudes of 80-85 km. The higher peak during summer is consistent with colder temperatures that cause faster chemical reactions of electron removal. By adopting temperature dependent empirical recombination rates from rocket experiments and meteor electron densities of 2×105-2×106 cm-3 in a decay time model, we are able to account for decreasing decay times below the peak for all seasons without invoking meteor electron removal by hypothetical icy particles.

Radiative decay of neutron-unbound intruder states in 19O

NASA Astrophysics Data System (ADS)

Dungan, R.; Tabor, S. L.; Tripathi, Vandana; Volya, A.; Kravvaris, K.; Abromeit, B.; Caussyn, D. D.; Morrow, S.; Parker, J. J.; Tai, P.-L.; VonMoss, J. M.

2016-02-01

The 9Be(14C, α γ ) reaction at EL a b=30 and 35 MeV was used to study excited states of 19O. The Florida State University (FSU) γ detector array was used to detect γ radiation in coincidence with charged particles detected and identified with a silicon Δ E -E particle telescope. γ decays have been observed for the first time from six states ranging from 368 to 2147 keV above the neutron separation energy (Sn=3962 keV) in 19O. The γ -decaying states are interspersed among states previously observed to decay by neutron emission. The ability of electromagnetic decay to compete successfully with neutron decay is explained in terms of neutron angular momentum barriers and small spectroscopic factors implying higher spin and complex structure for these intruder states. These results illustrate the need for complementary experimental approaches to best illuminate the complete nuclear structure.

Is there a relationship between the presence of the binary toxin genes in Clostridium difficile strains and the severity of C. difficile infection (CDI)?

PubMed

Berry, C E; Davies, K A; Owens, D W; Wilcox, M H

2017-12-01

Some strains of Clostridium difficile produce a binary toxin, in addition to the main C. difficile virulence factors (toxins A and B). There have been conflicting reports regarding the role of binary toxin and its relationship to the severity of C. difficile infection (CDI). Samples, isolates and clinical data were collected as part of a prospective multicentre diagnostic study. Clostridium difficile isolates (n = 1259) were tested by polymerase chain reaction (PCR) assay to detect binary toxin genes cdtA and cdtB. The PCR binary toxin gene results were compared with clinical severity and outcome data, including 30-day all-cause mortality. The 1259 isolates corresponded to 1083 different patients (October 2010 to September 2011). The prevalence of binary toxin positive strains was significantly higher in faecal samples with detectable toxin A/B than in those without toxin but that were positive by cytotoxigenic culture (26.3% vs. 10.3%, p < 0.001). The presence of binary toxin correlated moderately with markers of CDI severity (white cell count, serum albumin concentration and serum creatinine concentration). However, the risk ratio for all-cause mortality was 1.68 for binary toxin positive patients and patients were significantly less likely to survive if they had CDI caused by a binary toxin gene positive strain, even after adjusting for age (p < 0.001). The presence of binary toxin genes does not predict the clinical severity of CDI, but it is significantly associated with the risk of all-cause mortality.

Exponential Decay of Reconstruction Error from Binary Measurements of Sparse Signals

DTIC Science & Technology

2014-08-01

that the required condition of Corollary 9, namely q ≥ Cδ−4s̃ log(n/s̃), is still satisfied. The result follows from massaging the equations, as...study of the relationship of heart attacks to various factors may test whether certain subjects have heart attacks in a short window of time and other...subjects have heart attacks in a long window of time. The main message of this paper is that by carefully choosing this threshold the accuracy of

Multialternative drift-diffusion model predicts the relationship between visual fixations and choice in value-based decisions.

PubMed

Krajbich, Ian; Rangel, Antonio

2011-08-16

How do we make decisions when confronted with several alternatives (e.g., on a supermarket shelf)? Previous work has shown that accumulator models, such as the drift-diffusion model, can provide accurate descriptions of the psychometric data for binary value-based choices, and that the choice process is guided by visual attention. However, the computational processes used to make choices in more complicated situations involving three or more options are unknown. We propose a model of trinary value-based choice that generalizes what is known about binary choice, and test it using an eye-tracking experiment. We find that the model provides a quantitatively accurate description of the relationship between choice, reaction time, and visual fixation data using the same parameters that were estimated in previous work on binary choice. Our findings suggest that the brain uses similar computational processes to make binary and trinary choices.

Interrogation of bimetallic particle oxidation in three dimensions at the nanoscale

PubMed Central

Han, Lili; Meng, Qingping; Wang, Deli; Zhu, Yimei; Wang, Jie; Du, Xiwen; Stach, Eric A.; Xin, Huolin L.

2016-01-01

An understanding of bimetallic alloy oxidation is key to the design of hollow-structured binary oxides and the optimization of their catalytic performance. However, one roadblock encountered in studying these binary oxide systems is the difficulty in describing the heterogeneities that occur in both structure and chemistry as a function of reaction coordinate. This is due to the complexity of the three-dimensional mosaic patterns that occur in these heterogeneous binary systems. By combining real-time imaging and chemical-sensitive electron tomography, we show that it is possible to characterize these systems with simultaneous nanoscale and chemical detail. We find that there is oxidation-induced chemical segregation occurring on both external and internal surfaces. Additionally, there is another layer of complexity that occurs during the oxidation, namely that the morphology of the initial oxide surface can change the oxidation modality. This work characterizes the pathways that can control the morphology in binary oxide materials. PMID:27928998

Compound-nuclear Reactions with Unstable Isotopes: Constraining Capture Cross Sections with Indirect Data and Theory

NASA Astrophysics Data System (ADS)

Escher, Jutta

2016-09-01

Cross sections for compound-nuclear reactions involving unstable targets are important for many applications, but can often not be measured directly. Several indirect methods have recently been proposed to determine neutron capture cross sections for unstable isotopes. These methods aim at constraining statistical calculations of capture cross sections with data obtained from the decay of the compound nucleus relevant to the desired reaction. Each method produces this compound nucleus in a different manner (via a light-ion reaction, a photon-induced reaction, or β decay) and requires additional ingredients to yield the sought-after cross section. This contribution focuses on the process of determining capture cross sections from inelastic scattering and transfer experiments. Specifically, theoretical descriptions of the (p,d) transfer reaction have been developed to complement recent measurements in the Zr-Y region. The procedure for obtaining constraints for unknown capture cross sections is illustrated. The main advantages and challenges of this approach are compared to those of the proposed alternatives. This work is performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

Background studies of high energy γ rays from (n,γ) reactions in the CANDLES experiment

NASA Astrophysics Data System (ADS)

Nakajima, K.; Iida, T.; Akutagawa, K.; Batpurev, T.; Chan, W. M.; Dokaku, F.; Fushimi, K.; Kakubata, H.; Kanagawa, K.; Katagiri, S.; Kawasaki, K.; Khai, B. T.; Kino, H.; Kinoshita, E.; Kishimoto, T.; Hazama, R.; Hiraoka, H.; Hiyama, T.; Ishikawa, M.; Li, X.; Maeda, T.; Matsuoka, K.; Moser, M.; Nomachi, M.; Ogawa, I.; Ohata, T.; Sato, H.; Shamoto, K.; Shimada, M.; Shokati, M.; Takahashi, N.; Takemoto, Y.; Takihira, Y.; Tamagawa, Y.; Tozawa, M.; Teranishi, K.; Tetsuno, K.; Trang, V. T. T.; Tsuzuki, M.; Umehara, S.; Wang, W.; Yoshida, S.; Yotsunaga, N.

2018-07-01

High energy γ rays with several MeV produced by (n,γ) reactions can be a trouble for low background measurements in the underground laboratories such as double beta decay experiments. In the CANDLES project, which aimed to observe the neutrino-less double beta decay from 48Ca, γ rays caused by (n,γ) reactions were found to be the most significant background. The profile of the background was studied by measurements with a neutron source and a simulation with a validity check of neutron processes in Geant4. The observed spectrum of γ rays from (n,γ) reactions was well reproduced by the simulated spectra, which were originated from the surrounding rock and a detector tank made of stainless steel. The environmental neutron flux was derived by the observed event rate of γ rays from (n,γ) reactions using the simulation. The thermal and non-thermal neutron flux were found to be (1.3 ± 0.6) ×10-6 cm-2s-1 and (1.1 ± 0.5) ×10-5 cm-2s-1 , respectively. It is necessary to install an additional shield to reduce the background from (n,γ) reaction to the required level.

Open charm yields in d+Au collisions at squareroot[sNN]=200 GeV.

PubMed

Adams, J; Aggarwal, M M; Ahammed, Z; Amonett, J; Anderson, B D; Arkhipkin, D; Averichev, G S; Badyal, S K; Bai, Y; Balewski, J; Barannikova, O; Barnby, L S; Baudot, J; Bekele, S; Belaga, V V; Bellwied, R; Berger, J; Bezverkhny, B I; Bharadwaj, S; Bhasin, A; Bhati, A K; Bhatia, V S; Bichsel, H; Billmeier, A; Bland, L C; Blyth, C O; Bonner, B E; Botje, M; Boucham, A; Brandin, A V; Bravar, A; Bystersky, M; Cadman, R V; Cai, X Z; Caines, H; Calderón de la Barca Sánchez, M; Castillo, J; Cebra, D; Chajecki, Z; Chaloupka, P; Chattopadhyay, S; Chen, H F; Chen, Y; Cheng, J; Cherney, M; Chikanian, A; Christie, W; Coffin, J P; Cormier, T M; Cramer, J G; Crawford, H J; Das, D; Das, S; de Moura, M M; Derevschikov, A A; Didenko, L; Dietel, T; Dogra, S M; Dong, W J; Dong, X; Draper, J E; Du, F; Dubey, A K; Dunin, V B; Dunlop, J C; Dutta Mazumdar, M R; Eckardt, V; Edwards, W R; Efimov, L G; Emelianov, V; Engelage, J; Eppley, G; Erazmus, B; Estienne, M; Fachini, P; Faivre, J; Fatemi, R; Fedorisin, J; Filimonov, K; Filip, P; Finch, E; Fine, V; Fisyak, Y; Fomenko, K; Fu, J; Gagliardi, C A; Gaillard, L; Gans, J; Ganti, M S; Gaudichet, L; Geurts, F; Ghazikhanian, V; Ghosh, P; Gonzalez, J E; Grachov, O; Grebenyuk, O; Grosnick, D; Guertin, S M; Guo, Y; Gupta, A; Gutierrez, T D; Hallman, T J; Hamed, A; Hardtke, D; Harris, J W; Heinz, M; Henry, T W; Hepplemann, S; Hippolyte, B; Hirsch, A; Hjort, E; Hoffmann, G W; Huang, H Z; Huang, S L; Hughes, E W; Humanic, T J; Igo, G; Ishihara, A; Jacobs, P; Jacobs, W W; Janik, M; Jiang, H; Jones, P G; Judd, E G; Kabana, S; Kang, K; Kaplan, M; Keane, D; Khodyrev, V Yu; Kiryluk, J; Kisiel, A; Kislov, E M; Klay, J; Klein, S R; Koetke, D D; Kollegger, T; Kopytine, M; Kotchenda, L; Kramer, M; Kravtsov, P; Kravtsov, V I; Krueger, K; Kuhn, C; Kulikov, A I; Kumar, A; Kutuev, R Kh; Kuznetsov, A A; Lamont, M A C; Landgraf, J M; Lange, S; Laue, F; Lauret, J; Lebedev, A; Lednicky, R; Lehocka, S; LeVine, M J; Li, C; Li, Q; Li, Y; Lin, G; Lindenbaum, S J; Lisa, M A; Liu, F; Liu, L; Liu, Q J; Liu, Z; Ljubicic, T; Llope, W J; Long, H; Longacre, R S; Lopez-Noriega, M; Love, W A; Lu, Y; Ludlam, T; Lynn, D; Ma, G L; Ma, J G; Ma, Y G; Magestro, D; Mahajan, S; Mahapatra, D P; Majka, R; Mangotra, L K; Manweiler, R; Margetis, S; Markert, C; Martin, L; Marx, J N; Matis, H S; Matulenko, Yu A; McClain, C J; McShane, T S; Meissner, F; Melnick, Yu; Meschanin, A; Miller, M L; Minaev, N G; Mironov, C; Mischke, A; Mishra, D K; Mitchell, J; Mohanty, B; Molnar, L; Moore, C F; Morozov, D A; Munhoz, M G; Nandi, B K; Nayak, S K; Nayak, T K; Nelson, J M; Netrakanti, P K; Nikitin, V A; Nogach, L V; Nurushev, S B; Odyniec, G; Ogawa, A; Okorokov, V; Oldenburg, M; Olson, D; Pal, S K; Panebratsev, Y; Panitkin, S Y; Pavlinov, A I; Pawlak, T; Peitzmann, T; Perevoztchikov, V; Perkins, C; Peryt, W; Petrov, V A; Phatak, S C; Picha, R; Planinic, M; Pluta, J; Porile, N; Porter, J; Poskanzer, A M; Potekhin, M; Potrebenikova, E; Potukuchi, B V K S; Prindle, D; Pruneau, C; Putschke, J; Rakness, G; Raniwala, R; Raniwala, S; Ravel, O; Ray, R L; Razin, S V; Reichhold, D; Reid, J G; Renault, G; Retiere, F; Ridiger, A; Ritter, H G; Roberts, J B; Rogachevskiy, O V; Romero, J L; Rose, A; Roy, C; Ruan, L; Sahoo, R; Sakrejda, I; Salur, S; Sandweiss, J; Sarsour, M; Savin, I; Sazhin, P S; Schambach, J; Scharenberg, R P; Schmitz, N; Schweda, K; Seger, J; Seyboth, P; Shahaliev, E; Shao, M; Shao, W; Sharma, M; Shen, W Q; Shestermanov, K E; Shimanskiy, S S; Sichtermann, E; Simon, F; Singaraju, R N; Skoro, G; Smirnov, N; Snellings, R; Sood, G; Sorensen, P; Sowinski, J; Speltz, J; Spinka, H M; Srivastava, B; Stadnik, A; Stanislaus, T D S; Stock, R; Stolpovsky, A; Strikhanov, M; Stringfellow, B; Suaide, A A P; Sugarbaker, E; Suire, C; Sumbera, M; Surrow, B; Symons, T J M; Szanto de Toledo, A; Szarwas, P; Tai, A; Takahashi, J; Tang, A H; Tarnowsky, T; Thein, D; Thomas, J H; Timoshenko, S; Tokarev, M; Trainor, T A; Trentalange, S; Tribble, R E; Tsai, O D; Ulery, J; Ullrich, T; Underwood, D G; Urkinbaev, A; Van Buren, G; van Leeuwen, M; Vander Molen, A M; Varma, R; Vasilevski, I M; Vasiliev, A N; Vernet, R; Vigdor, S E; Viyogi, Y P; Vokal, S; Voloshin, S A; Vznuzdaev, M; Waggoner, W T; Wang, F; Wang, G; Wang, G; Wang, X L; Wang, Y; Wang, Y; Wang, Z M; Ward, H; Watson, J W; Webb, J C; Wells, R; Westfall, G D; Wetzler, A; Whitten, C; Wieman, H; Wissink, S W; Witt, R; Wood, J; Wu, J; Xu, N; Xu, Z; Xu, Z Z; Yamamoto, E; Yepes, P; Yurevich, V I; Zanevsky, Y V; Zhang, H; Zhang, W M; Zhang, Z P; Zoulkarneev, R; Zoulkarneeva, Y; Zubarev, A N

2005-02-18

Midrapidity open charm spectra from direct reconstruction of D0(D0)-->K-/+pi+/- in d+Au collisions and indirect electron-positron measurements via charm semileptonic decays in p+p and d+Au collisions at squareroot[sNN]=200 GeV are reported. The D0(D0) spectrum covers a transverse momentum (pT) range of 0.1

Probing the neutron star spin evolution in the young Small Magellanic Cloud Be/X-ray binary SXP 1062

NASA Astrophysics Data System (ADS)

Popov, S. B.; Turolla, R.

2012-03-01

The newly discovered Be/X-ray binary in the Small Magellanic Cloud, SXP 1062, provides the first example of a robust association with a supernova remnant (SNR). The short age estimated for the SNR qualifies SXP 1062 as the youngest known source in its class, ?. As such, it allows us to test current models of magnetorotational evolution of neutron stars in a still unexplored regime. Here we discuss possible evolutionary scenarios for SXP 1062 in an attempt to reconcile its long spin period, ?, and short age. Although several options can be considered, like an anomalously long initial period or the presence of a fossil disc, our results indicate that SXP 1062 may host a neutron star born with a large initial magnetic field, typically in excess of ˜ 1014 G, which then decayed to ˜ 1013 G.

Double charmonia production in exclusive Z-boson decays

NASA Astrophysics Data System (ADS)

Likhoded, A. K.; Luchinsky, A. V.

2018-05-01

This paper is devoted to systematic analysis of double charmonium production in exclusive Z-boson decays in the framework of non-relativistic quantum chromodynamics (NRQCD) and leading twist light-cone (LC) models. Theoretical predictions for branching fractions of all considered decays are presented. According to the obtained results in the case of the allowed helicity suppression rule processes, the effect of internal quark motion increases the branching fractions by a factor 1.5, while for forbidden reactions the LC predictions are strictly zero, while NRQCD ones are significantly smaller than for allowed.

Selected spectroscopic results on element 115 decay chains

DOE PAGES

Rudolph, D.; Forsberg, U.; Golubev, P.; ...

2014-08-24

We observed thirty correlated α-decay chains in an experiment studying the fusion-evaporation reaction 48Ca + 243Am at the GSI Helmholtzzentrum fur Schwerionenforschung. The decay characteristics of the majority of these 30 chains are consistent with previous observations and interpretations of such chains to originate from isotopes of element Z = 115. High-resolution α-photon coincidence spectroscopy in conjunction with comprehensive Monte-Carlo simulations allow to propose excitation schemes of atomic nuclei of the heaviest elements, thereby probing nuclear structure models near the 'Island of Stability' with unprecedented experimental precision.

Surface-promoted hydrolysis of 2,4,6-trinitrotoluene and 2,4-dinitroanisole on pyrogenic carbonaceous matter.

PubMed

Ding, Kai; Byrnes, Cory; Bridge, Jarrod; Grannas, Amanda; Xu, Wenqing

2018-04-01

This study investigates the fate of sorbed nitroaromatics on the surface of pyrogenic carbonaceous matter (PCM) to assess the feasibility of a PCM-promoted hydrolysis. The degradation of two nitroaromatic compounds, 2,4,6-trinitrotoluene (TNT) and 2,4-dinitroanisole, was observed at pH 7 in the presence of graphite powder, a model PCM. By contrast, no decay occurred without graphite. Using TNT as a model compound, our results suggest that TNT decay demonstrated a strong pH dependence, with no reaction at pH 3-5 but rapid degradation at pH 6-10. Moreover, by fitting TNT decay at different pH conditions along with its sorption kinetics to the Langmuir Kinetic Model, our results suggest that the base-catalyzed hydrolysis was important. The activation energy for TNT decay was obtained by measuring reaction rates at different temperatures with or without graphite and no significant difference was observed. However, the addition of tetramethylammonium cation was able to promote TNT decay possibly due to its ability to attract more OH - from the aqueous solution, leading to an increase in the sorbed OH - concentrations. Nitrite and a Meisenheimer complex were identified as degradation products for TNT. Other PCM, such as biochar, also demonstrated a comparable ability in promoting TNT decay at pH 7. Furthermore, a rapid degradation of TNT at pH 7 was observed when biochar was used as a soil amendment (4% by weight). Our results suggest that PCM can facilitate TNT and 2,4-dinitroanisole decay via a surface-promoted hydrolysis at neutral pH conditions, suggesting a promising alternative for in situ soil remediation. Copyright © 2018 Elsevier Ltd. All rights reserved.

IAEA Co-ordinated Research Project: update of X-ray and gamma-ray decay data standards for detector calibration and other applications.

PubMed

Nichols, Alan L

2004-01-01

A Co-ordinated Research Project (CRP) was established in 1998 by the IAEA Nuclear Data Section (Update of X-ray and gamma-ray Decay Data Standards for Detector Calibration and Other Applications), in order to improve further the recommended decay data used to undertake efficiency calibrations of gamma-ray detectors. Participants in this CRP reviewed and modified the list of radionuclides most suited for detector efficiency calibration, and also considered the decay-data needs for safeguards, waste management, dosimetry, nuclear medicine, material analysis and environmental monitoring. Overall, 62 radionuclides were selected for decay-data evaluation, along with four parent-daughter combinations and two natural decay chains. gamma-ray emissions from specific nuclear reactions were also included to extend the calibrant energy well beyond 10 MeV. A significant number of these decay-data evaluations have been completed, and an IAEA-TECDOC report and database are in the process of being assembled for planned completion by the end of 2003.

Binary toxin and its clinical importance in Clostridium difficile infection, Belgium.

PubMed

Pilate, T; Verhaegen, J; Van Ranst, M; Saegeman, V

2016-11-01

Binary toxin-producing Clostridium difficile strains such as ribotypes 027 and 078 have been associated with increased Clostridium difficile infection (CDI) severity. Our objective was to investigate the association between presence of the binary toxin gene and CDI severity and recurrence. We performed a laboratory-based retrospective study including patients between January 2013 and March 2015 whose fecal samples were analyzed by polymerase chain reaction (PCR) for the presence of the genes for toxin B and binary toxin and a deletion in the tcdC gene, specific for ribotype 027. Clinical and epidemiological characteristics were compared between 33 binary toxin-positive CDI patients and 33 binary toxin-negative CDI patients. Subsequently, the characteristics of 66 CDI patients were compared to those of 66 diarrhea patients who were carriers of non-toxigenic C. difficile strains. Fifty-nine of 1034 (5.7 %) fecal samples analyzed by PCR were binary toxin-positive, belonging to 33 different patients. No samples were positive for ribotype 027. Binary toxin-positive CDI patients did not differ from binary toxin-negative CDI patients in terms of disease recurrence, morbidity, or mortality, except for a higher peripheral leukocytosis in the binary toxin-positive group (16.30 × 10 9 /L vs. 11.65 × 10 9 /L; p = 0.02). The second part of our study showed that CDI patients had more severe disease, but not a higher 30-day mortality rate than diarrhea patients with a non-toxicogenic C. difficile strain. In our setting with a low prevalence of ribotype 027, the presence of the binary toxin gene is not associated with poor outcome.

Transition metals and water-soluble ions in deposits on a building and their potential catalysis of stone decay

NASA Astrophysics Data System (ADS)

McAlister, J. J.; Smith, B. J.; Török, A.

Atmospheric particulates (dust) deposited on buildings are a complex chemical and mineralogical mixture including transition metal oxide matrices that act as a significant medium for further surface reactions and provide efficient sinks for pollutants, especially in urban environments. Once deposited, their transformation by reaction with specific and often highly localised environmental conditions across building facades is related to their degree of exposure to rain-wash. These transformations are central to the soiling of buildings and the availability of salts that lead to stone decay. To investigate these relationships, samples were collected at high and low elevations and under highly and moderately sheltered conditions from a building located on a busy arterial route in Budapest. Selective extraction analysis highlights the mobility/availability of Fe, Mn, Zn, Cu, Cr, Pb and Ni, plus water-soluble Ca 2+, Mg 2+, Na +, K +, Cl -, SO 42- and NO 3- and their potential to take part in surface reactions that could enhance stone decay. Concentrations of water-soluble Fe, Mn and Zn in sheltered dust reach 126 mg kg -1, 80 mg kg -1 and 220 mg kg -1 respectively and under acidic environmental conditions and high humidity, similar levels of Mn and significantly higher concentrations of Fe, Zn, Cu and Pb may be released from the exchangeable/carbonate phase making these metals potentially available to catalyse surface reactions. Sulphate and nitrate coatings plus sufficient moisture increase metal solubility and active sites may be regenerated allowing mobile transition metals to become available and possibly catalyse further surface reactions.

High Temperature Reactions of Uranium Dioxide with Various Metal Oxides

DTIC Science & Technology

1956-02-20

manganese, nickel , lead, and tin. Subtracting the total of these impurities from the oxygen remainder would give a more nearly 1:2 uranium -oxygen ratio. The...Astin, Dire~ctor High -Temperature Reactions of Uranium Dioxide With Various Metal Oxides Acceson For NTIS CRAWI DTfC TAB Unannounced D JustifiCation...1 2. The uranium -oxygen system ------------------------------------- 1 3. Binary systems containing

Synthesis and molecular structure of a spheroidal binary nanoscale copper sulfide cluster.

PubMed

Bestgen, Sebastian; Fuhr, Olaf; Roesky, Peter W; Fenske, Dieter

2016-09-27

The reaction of copper(4-(tert-butyl)phenyl)methanethiolate [CuSCH 2 C 6 H 4 t Bu] with bis(trimethylsilyl)sulfide S(SiMe 3 ) 2 in the presence of triphenylphosphine PPh 3 afforded the binary 52 nuclear copper cluster [Cu 52 S 12 (SCH 2 C 6 H 4 t Bu) 28 (PPh 3 ) 8 ]. The molecular structure of this intensely red coloured nanoscale Cu 2 S mimic was established by single crystal X-ray diffraction.

Enhanced chlorine dioxide decay in the presence of metal oxides: relevance to drinking water distribution systems.

PubMed

Liu, Chao; von Gunten, Urs; Croué, Jean-Philippe

2013-08-06

Chlorine dioxide (ClO2) decay in the presence of typical metal oxides occurring in distribution systems was investigated. Metal oxides generally enhanced ClO2 decay in a second-order process via three pathways: (1) catalytic disproportionation with equimolar formation of chlorite and chlorate, (2) reaction to chlorite and oxygen, and (3) oxidation of a metal in a reduced form (e.g., cuprous oxide) to a higher oxidation state. Cupric oxide (CuO) and nickel oxide (NiO) showed significantly stronger abilities than goethite (α-FeOOH) to catalyze the ClO2 disproportionation (pathway 1), which predominated at higher initial ClO2 concentrations (56-81 μM). At lower initial ClO2 concentrations (13-31 μM), pathway 2 also contributed. The CuO-enhanced ClO2 decay is a base-assisted reaction with a third-order rate constant of 1.5 × 10(6) M(-2) s(-1) in the presence of 0.1 g L(-1) CuO at 21 ± 1 °C, which is 4-5 orders of magnitude higher than in the absence of CuO. The presence of natural organic matter (NOM) significantly enhanced the formation of chlorite and decreased the ClO2 disproportionation in the CuO-ClO2 system, probably because of a higher reactivity of CuO-activated ClO2 with NOM. Furthermore, a kinetic model was developed to simulate CuO-enhanced ClO2 decay at various pH values. Model simulations that agree well with the experimental data include a pre-equilibrium step with the rapid formation of a complex, namely, CuO-activated Cl2O4. The reaction of this complex with OH(-) is the rate-limiting and pH-dependent step for the overall reaction, producing chlorite and an intermediate that further forms chlorate and oxygen in parallel. These novel findings suggest that the possible ClO2 loss and the formation of chlorite/chlorate should be carefully considered in drinking water distribution systems containing copper pipes.

Fast-neutron-induced potential background near the Q value of neutrinoless double-β decay of 76Ge

NASA Astrophysics Data System (ADS)

Tornow, W.; Bhike, Megha; Fallin, B.; Krishichayan

2016-01-01

The 76Ge (n,p)76Ga reaction and the subsequent β decay of 76Ga to 76Ge has been used to excite the 3951.89-keV state of 76Ge , which decays by the emission of a 2040.70-keV γ ray. Using high-purity germanium detectors, the associated pulse-height signal may be undistinguishable from the potential signal produced in neutrinoless double-β decay of 76Ge with its Q value of 2039.0 keV. At 20-MeV neutron energy the production cross section of the 2040.70-keV γ ray is approximately 0.1 mb.

Accurate Waveforms for Non-spinning Binary Black Holes using the Effective-one-body Approach

NASA Technical Reports Server (NTRS)

Buonanno, Alessandra; Pan, Yi; Baker, John G.; Centrella, Joan; Kelly, Bernard J.; McWilliams, Sean T.; vanMeter, James R.

2007-01-01

Using numerical relativity as guidance and the natural flexibility of the effective-one-body (EOB) model, we extend the latter so that it can successfully match the numerical relativity waveforms of non-spinning binary black holes during the last stages of inspiral, merger and ringdown. Here, by successfully, we mean with phase differences < or approx. 8% of a gravitational-wave cycle accumulated until the end of the ringdown phase. We obtain this result by simply adding a 4 post-Newtonian order correction in the EOB radial potential and determining the (constant) coefficient by imposing high-matching performances with numerical waveforms of mass ratios m1/m2 = 1,2/3,1/2 and = 1/4, m1 and m2 being the individual black-hole masses. The final black-hole mass and spin predicted by the numerical simulations are used to determine the ringdown frequency and decay time of three quasi-normal-mode damped sinusoids that are attached to the EOB inspiral-(plunge) waveform at the light-ring. The accurate EOB waveforms may be employed for coherent searches of gravitational waves emitted by non-spinning coalescing binary black holes with ground-based laser-interferometer detectors.

Imprints of dynamical interactions on brown dwarf pairing statistics and kinematics

NASA Astrophysics Data System (ADS)

Sterzik, M. F.; Durisen, R. H.

2003-03-01

We present statistically robust predictions of brown dwarf properties arising from dynamical interactions during their early evolution in small clusters. Our conclusions are based on numerical calculations of the internal cluster dynamics as well as on Monte-Carlo models. Accounting for recent observational constraints on the sub-stellar mass function and initial properties in fragmenting star forming clumps, we derive multiplicity fractions, mass ratios, separation distributions, and velocity dispersions. We compare them with observations of brown dwarfs in the field and in young clusters. Observed brown dwarf companion fractions around 15 +/- 7% for very low-mass stars as reported recently by Close et al. (\\cite{CSFB03}) are consistent with certain dynamical decay models. A significantly smaller mean separation distribution for brown dwarf binaries than for binaries of late-type stars can be explained by similar specific energy at the time of cluster formation for all cluster masses. Due to their higher velocity dispersions, brown-dwarfs and low-mass single stars will undergo time-dependent spatial segregation from higher-mass stars and multiple systems. This will cause mass functions and binary statistics in star forming regions to vary with the age of the region and the volume sampled.

A Periodically Varying Luminous Quasar at z = 2 from the Pan-STARRS1 Medium Deep Survey: A Candidate Supermassive Black Hole Binary in the Gravitational Wave-Driven Regime

NASA Astrophysics Data System (ADS)

Liu, Tingting; Gezari, Suvi

Supermassive black hole binaries (SMBHBs) should be an inevitable consequence of the hierarchical growth of massive galaxies through mergers and the strongest sirens of gravitational waves (GWs) in the cosmos. Yet, their direct detection has remained elusive due to the compact (sub-parsec) orbital separations of gravitationally bound SMBHBs. Here we exploit a theoretically predicted signature of SMBHBs in the time domain. We have begun a systematic search for SMBHB candidates in the Pan-STARRS1 Medium Deep Survey (MDS) and reported our first significant detection of such a candidate from our pilot study of MD09 in Liu et al. (2015). Our candidate PSO J334.2028+01.4075 has a detected period of 542 days, varying persistently over the available baseline. From its archival spectrum, we estimated the black hole mass of the z = 2.06 quasar to be ~1010 M⊙. The inferred ~7 R s binary separation therefore puts this candidate in the regime of GW-dominated orbital decay, opening up the exciting possibility of finding GW sources detectable by pulsar timing arrays (PTAs) in a wide-field optical synoptic survey.

Decoding Mode-mixing in Black-hole Merger Ringdown

NASA Technical Reports Server (NTRS)

Kelly, Bernard J.; Baker, John G.

2013-01-01

Optimal extraction of information from gravitational-wave observations of binary black-hole coalescences requires detailed knowledge of the waveforms. Current approaches for representing waveform information are based on spin-weighted spherical harmonic decomposition. Higher-order harmonic modes carrying a few percent of the total power output near merger can supply information critical to determining intrinsic and extrinsic parameters of the binary. One obstacle to constructing a full multi-mode template of merger waveforms is the apparently complicated behavior of some of these modes; instead of settling down to a simple quasinormal frequency with decaying amplitude, some |m| = modes show periodic bumps characteristic of mode-mixing. We analyze the strongest of these modes the anomalous (3, 2) harmonic mode measured in a set of binary black-hole merger waveform simulations, and show that to leading order, they are due to a mismatch between the spherical harmonic basis used for extraction in 3D numerical relativity simulations, and the spheroidal harmonics adapted to the perturbation theory of Kerr black holes. Other causes of mode-mixing arising from gauge ambiguities and physical properties of the quasinormal ringdown modes are also considered and found to be small for the waveforms studied here.

COAL/POLYMER COPROCESSING WITH EFFICIENT USE OF HYDROGEN

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dr. Linda J. Broadbelt; Matthew J. DeWitt; Hsi-Wu Wong

2000-09-30

The final project period was devoted to investigating the binary mixture pyrolysis of polypropylene and polystyrene. Their interactions were assessed in order to provide a baseline for experiments with multicomponent mixtures of polymers with coal. Pyrolysis of polypropylene, polystyrene and their binary mixture was investigated at temperatures of 350 C and 420 C with reaction times from 1 to 180 minutes. Two different loadings, 10 mg and 20 mg, were studied for neat polypropylene and polystyrene to assess the effect of total pressure on product yields and selectivities. For neat pyrolysis of polypropylene, total conversion was much higher at 420more » C, and no significant effect of loading on the total conversion was observed. Four classes of products, alkanes, alkenes, dienes, and aromatic compounds, were observed, and their distribution was explained by a typical free radical mechanism. For neat polystyrene pyrolysis, conversion reached approximately 75% at 350 C, while at 420 C the conversion reached a maximum around 90% at 10 minutes and decreased at longer times because of condensation reactions. The selectivities to major products were slightly different for the two different loadings due to the effect of total reaction pressure on secondary reactions. For binary mixture pyrolysis, the overall conversion was higher than the average of the two neat cases. The conversion of polystyrene remained the same, but a significant enhancement in the polypropylene conversion was observed. This suggests that the less reactive polypropylene was initiated by polystyrene-derived radicals. These results are summarized in detail in an attached manuscript that is currently in preparation. The other results obtained during the lifetime of this grant are documented in the set of attached manuscripts.« less

Study of complexation process between 4'-nitrobenzo-15-crown-5 and yttrium(III) cation in binary mixed non-aqueous solvents using conductometric method

NASA Astrophysics Data System (ADS)

Habibi, N.; Rounaghi, G. H.; Mohajeri, M.

2012-12-01

The complexation reaction of macrocyclic ligand (4'-nitrobenzo-15C5) with Y3+ cation was studied in acetonitrile-methanol (AN-MeOH), acetonitrile-ethanol (AN-EtOH), acetonitrile-dimethylformamide (AN-DMF) and ethylacetate-methanol (EtOAc-MeOH) binary mixtures at different temperatures using conductometry method. The conductivity data show that in all solvent systems, the stoichiometry of the complex formed between 4'-nitrobenzo-15C5 and Y3+ cation is 1: 1 (ML). The stability order of (4'-nitrobenzo-15C5). Y3+ complex in pure non-aqueous solvents at 25°C was found to be: EtOAc > EtOH > AN ≈ DMF > MeOH, and in the case of most compositions of the binary mixed solvents at 25°C it was: AN≈MeOH ≈ AN-EtOH > AN-DMF > EtOAc-MeOH. But the results indicate that the sequence of the stability of the complex in the binary mixed solutions changes with temperature. A non-linear behavior was observed for changes of log K f of (4'-nitrobenzo-15C5 · Y3+) complex versus the composition of the binary mixed solvents, which was explained in terms of solvent-solvent interactions and also the hetero-selective solvation of the species involved in the complexation reaction. The values of thermodynamic parameters (Δ H {c/ℴ} and Δ S {c/ℴ}) for formation of the complex were obtained from temperature dependent of the stability constant using the van't Hoff plots. The results represent that in most cases, the complex is both enthalpy and entropy stabilized and the values and also the sign of thermodynamic parameters are influenced by the nature and composition of the mixed solvents.

Reaction of maturity group V soybean plant introductions to Phomopsis Seed Decay in Arkansas Mississippi and Missouri 2009

USDA-ARS?s Scientific Manuscript database

In 2009, Soybean Phomopsis seed decay (PSD) caused over 12 million bushels of yield loss in 16 southern states. This disease severely affects soybean seed quality due to the reduction of seed viability, oil content, and alteration of seed composition, and it may also increase moldy and/or split seed...

A new assessment of the alleged link between element 115 and element 117 decay chains

NASA Astrophysics Data System (ADS)

Forsberg, U.; Rudolph, D.; Fahlander, C.; Golubev, P.; Sarmiento, L. G.; Åberg, S.; Block, M.; Düllmann, Ch. E.; Heßberger, F. P.; Kratz, J. V.; Yakushev, A.

2016-09-01

A novel rigorous statistical treatment is applied to available data (May 9, 2016) from search and spectroscopy experiments on the elements with atomic numbers Z = 115 and Z = 117. The present analysis implies that the hitherto proposed cross-reaction link between α-decay chains associated with the isotopes 293117 and 289115 is highly improbable.

Nuclear Data Sheets for A = 136

NASA Astrophysics Data System (ADS)

Sonzogni, A. A.

2002-04-01

Experimental data on ground-- and excited--state properties for all known nuclei with mass number A=136 have been compiled and evaluated. States populated in radioactive decay as well as in nuclear reactions have been considered. For these nuclei, level and decay schemes, as well as tables of nuclear properties are presented. This work supersedes the 1994 evaluation by J.K. Tuli (1994Tu01).

Rapid reaction of nanomolar Mn(II) with superoxide radical in seawater and simulated freshwater

USGS Publications Warehouse

Hansard, S.P.; Easter, H.D.; Voelker, Bettina M.

2011-01-01

Superoxide radical (O2-) has been proposed to be an important participant in oxidation-reduction reactions of metal ions in natural waters. Here, we studied the reaction of nanomolar Mn(II) with O 2- in seawater and simulated freshwater, using chemiluminescence detection of O2- to quantify the effect of Mn(II) on the decay kinetics of O2-. With 3-24 nM added [Mn(II)] and <0.7 nM [O2-], we observed effective second-order rate constants for the reaction of Mn(II) with O2- of 6 ?? 106 to 1 ?? 107 M -1???s-1 in various seawater samples. In simulated freshwater (pH 8.6), the effective rate constant of Mn(II) reaction with O 2- was somewhat lower, 1.6 ?? 106 M -1???s-1. With higher initial [O2-], in excess of added [Mn(II)], catalytic decay of O 2- by Mn was observed, implying that a Mn(II/III) redox cycle occurred. Our results show that reactions with nanomolar Mn(II) could be an important sink of O2- in natural waters. In addition, reaction of Mn(II) with superoxide could maintain a significant fraction of dissolved Mn in the +III oxidation state. ?? 2011 American Chemical Society.

Spreading out of perturbations in reversible reaction networks

NASA Astrophysics Data System (ADS)

Maslov, Sergei; Sneppen, Kim; Ispolatov, I.

2007-08-01

Using an example of physical interactions between proteins, we study how a perturbation propagates in the equilibrium of a network of reversible reactions governed by the law of mass action. We introduce a matrix formalism to describe the linear response of all equilibrium concentrations to shifts in total abundances of individual reactants, and reveal its heuristic analogy to the flow of electric current in a network of resistors. Our main conclusion is that, on average, the induced changes in equilibrium concentrations decay exponentially as a function of network distance from the source of perturbation. We analyze how this decay is influenced by such factors as the topology of a network, binding strength, and correlations between concentrations of neighboring nodes. We find that the minimal branching of the network, small values of dissociation constants, and low equilibrium free (unbound) concentrations of reacting substances all decrease the decay constant and thus increase the range of propagation. Exact analytic expressions for the decay constant are obtained for the case of equally strong interactions and uniform as well as oscillating concentrations on the Bethe lattice. Our general findings are illustrated using a real network of protein-protein interactions in baker's yeast with experimentally determined protein concentrations.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gates, J. M.; Gregorich, K. E.; Gothe, O. R.

In this study, forty-six decay chains, assigned to the decay of 288115, were produced using the 243Am ( 48Ca, 3n) 288115 reaction at the Lawrence Berkeley National Laboratory 88-in. cyclotron. The resulting series of α decays were studied using α-photon and α-x-ray spectroscopies. Multiple α-photon coincidences were observed in the element 115 decay chain members, particularly in the third- and fourth-generation decays (presumed to be 280Rg and 276Mt, respectively). Upon combining these data with those from 22 288115 decay chains observed in a similar experiment, updated level schemes in 276Mt and 272Bh (populated by the α decay of 280Rg andmore » 276Mt, respectively) are proposed. Additionally, photons were observed in the energy range expected for K x rays coincident with the α decay of both 280Rg and 276Mt. However, Compton scattering of higher-energy γ rays and discrete transitions are present in the K x-ray region preventing a definitive Z identification to be made based on observation of characteristic K x-ray energies.« less

Hydrodynamical processes in coalescing binary stars

NASA Astrophysics Data System (ADS)

Lai, Dong

1994-01-01

Coalescing neutron star binaries are considered to be the most promising sources of gravitational waves that could be detected by the planned laser-interferometer LIGO/VIRGO detectors. Extracting gravity wave signals from noisy data requires accurate theoretical waveforms in the frequency range 10-1000 Hz end detailed understanding of the dynamics of the binary orbits. We investigate the quasi-equilibrium and dynamical tidal interactions in coalescing binary stars, with particular focus on binary neutron stars. We develop a new formalism to study the equilibrium and dynamics of fluid stars in binary systems. The stars are modeled as compressible ellipsoids, and satisfy polytropic equation of state. The hydrodynamic equations are reduced to a set of ordinary differential equations for the evolution of the principal axes and other global quantities. The equilibrium binary structure is determined by a set of algebraic equations. We consider both synchronized and nonsynchronized systems, obtaining the generalizations to compressible fluid of the classical results for the ellipsoidal binary configurations. Our method can be applied to a wide variety of astrophysical binary systems containing neutron stars, white dwarfs, main-sequence stars and planets. We find that both secular and dynamical instabilities can develop in close binaries. The quasi-static (secular) orbital evolution, as well as the dynamical evolution of binaries driven by viscous dissipation and gravitational radiation reaction are studied. The development of the dynamical instability accelerates the binary coalescence at small separation, leading to appreciable radial infall velocity near contact. We also study resonant excitations of g-mode oscillations in coalescing binary neutron stars. A resonance occurs when the frequency of the tidal driving force equals one of the intrinsic g-mode frequencies. Using realistic microscopic nuclear equations of state, we determine the g-modes in a cold neutron atar. Resonant excitations of these g-modes during the last few minutes of the binary coalescence result in energy transfer and angular momentum transfer from the binary orbit to the neutron star. Because of the weak coupling between the g-modes and the tidal potential, the induced orbital phase errors due to resonances are small. However, resonant excitations of the g-modes play an important role in the tidal heating of binary neutron stars.

Controlling behavioral experiments with a new programming language (SORCA) for microcomputer systems.

PubMed

Brinkhus, H B; Klinkenborg, H; Estorf, R; Weber, R

1983-01-01

A new programming language SORCA has been defined and a compiler has been written for Z80-based microcomputer systems with CP/M operating system. The language was developed to control behavioral experiments by external stimuli and by time schedule in real-time. Eight binary hardware input lines are sampled cyclically by the computer and can be used to sense switches, level detectors and other binary information, while 8 binary hardware output lines, that are cyclically updated, can be used to control relays, lamps, generate tones or for other purposes. The typical reaction time (cycle time) of a SORCA-program is 500 microseconds to 1 ms. All functions can be programmed as often as necessary. Included are the basic logic functions, counters, timers, majority gates and other complex functions. Parameters can be given as constants or as a result of a step function or of a random process (with Gaussian or equal distribution). Several tasks can be performed simultaneously. In addition, results of an experiment (e.g., number of reactions or latencies) can be measured and printed out on request or automatically. The language is easy to learn and can also be used for many other control purposes.

Decay spectroscopy of element 115 daughters: Rg 280 → Mt 276 and Mt 276 → Bh 272

DOE PAGES

Gates, J. M.; Gregorich, K. E.; Gothe, O. R.; ...

2015-08-03

In this study, forty-six decay chains, assigned to the decay of 288115, were produced using the 243Am ( 48Ca, 3n) 288115 reaction at the Lawrence Berkeley National Laboratory 88-in. cyclotron. The resulting series of α decays were studied using α-photon and α-x-ray spectroscopies. Multiple α-photon coincidences were observed in the element 115 decay chain members, particularly in the third- and fourth-generation decays (presumed to be 280Rg and 276Mt, respectively). Upon combining these data with those from 22 288115 decay chains observed in a similar experiment, updated level schemes in 276Mt and 272Bh (populated by the α decay of 280Rg andmore » 276Mt, respectively) are proposed. Additionally, photons were observed in the energy range expected for K x rays coincident with the α decay of both 280Rg and 276Mt. However, Compton scattering of higher-energy γ rays and discrete transitions are present in the K x-ray region preventing a definitive Z identification to be made based on observation of characteristic K x-ray energies.« less

Low-Frequency Gravitational Radiation from Coalescing Massive Black Hole Binaries in Hierarchical Cosmologies

NASA Astrophysics Data System (ADS)

Sesana, Alberto; Haardt, Francesco; Madau, Piero; Volonteri, Marta

2004-08-01

We compute the expected low-frequency gravitational wave signal from coalescing massive black hole (MBH) binaries at the center of galaxies in a hierarchical structure formation scenario in which seed holes of intermediate mass form far up in the dark halo ``merger tree.'' The merger history of dark matter halos and associated MBHs is followed via cosmological Monte Carlo realizations of the merger hierarchy from redshift z=20 to the present in a ΛCDM cosmology. MBHs get incorporated through halo mergers into larger and larger structures, sink to the center because of dynamical friction against the dark matter background, accrete cold material in the merger remnant, and form MBH binary systems. Stellar dynamical (three-body) interactions cause the hardening of the binary at large separations, while gravitational wave emission takes over at small radii and leads to the final coalescence of the pair. A simple scheme is applied in which the ``loss cone'' is constantly refilled and a constant stellar density core forms because of the ejection of stars by the shrinking binary. The integrated emission from inspiraling MBH binaries at all redshifts is computed in the quadrupole approximation and results in a gravitational wave background (GWB) with a well-defined shape that reflects the different mechanisms driving the late orbital evolution. The characteristic strain spectrum has the standard hc(f)~f-2/3 behavior only in the range f=10-9to10-6 Hz. At lower frequencies the orbital decay of MBH binaries is driven by the ejection of background stars (``gravitational slingshot''), and the strain amplitude increases with frequency, hc(f)~f. In this range the GWB is dominated by 109-1010 Msolar MBH pairs coalescing at 0<~z<~2. At higher frequencies, f>10-6Hz, the strain amplitude, as steep as hc(f)~f-1.3, is shaped by the convolution of last stable circular orbit emission by lighter binaries (102-107 Msolar) populating galaxy halos at all redshifts. We discuss the observability of inspiraling MBH binaries by a low-frequency gravitational wave experiment such as the planned Laser Interferometer Space Antenna (LISA). Over a 3 yr observing period LISA should resolve this GWB into discrete sources, detecting ~60 (~250) individual events above an S/N=5 (S/N=1) confidence level.

Contributions to the NUCLEI SciDAC-3 Project

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bogner, Scott; Nazarewicz, Witek

This is the Final Report for Michigan State University for the NUCLEI SciDAC-3 project. The NUCLEI project, as defined by the scope of work, has developed, implemented and run codes for large-scale computations of many topics in low-energy nuclear physics. Physics studied included the properties of nuclei and nuclear decays, nuclear structure and reactions, and the properties of nuclear matter. The computational techniques used included Configuration Interaction, Coupled Cluster, and Density Functional methods. The research program emphasized areas of high interest to current and possible future DOE nuclear physics facilities, including ATLAS at ANL and FRIB at MSU (nuclear structuremore » and reactions, and nuclear astrophysics), TJNAF (neutron distributions in nuclei, few body systems, and electroweak processes), NIF (thermonuclear reactions), MAJORANA and FNPB (neutrinoless double-beta decay and physics beyond the Standard Model), and LANSCE (fission studies).« less

Nuclear Computational Low Energy Initiative (NUCLEI)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Reddy, Sanjay K.

This is the final report for University of Washington for the NUCLEI SciDAC-3. The NUCLEI -project, as defined by the scope of work, will develop, implement and run codes for large-scale computations of many topics in low-energy nuclear physics. Physics to be studied include the properties of nuclei and nuclear decays, nuclear structure and reactions, and the properties of nuclear matter. The computational techniques to be used include Quantum Monte Carlo, Configuration Interaction, Coupled Cluster, and Density Functional methods. The research program will emphasize areas of high interest to current and possible future DOE nuclear physics facilities, including ATLAS andmore » FRIB (nuclear structure and reactions, and nuclear astrophysics), TJNAF (neutron distributions in nuclei, few body systems, and electroweak processes), NIF (thermonuclear reactions), MAJORANA and FNPB (neutrino-less double-beta decay and physics beyond the Standard Model), and LANSCE (fission studies).« less

MODELING CHLORINE RESIDUALS IN DRINKING-WATER DISTRIBUTION SYSTEMS

EPA Science Inventory

A mass-transfer-based model is developed for predicting chlorine decay in drinking-water distribution networks. The model considers first-order reactions of chlorine to occur both in the bulk flow and at the pipe wall. The overall rate of the wall reaction is a function of the ...

MODELING CHLORINE RESIDUALS IN DRINKING-WATER DISTRIBUTION SYSTEMS

EPA Science Inventory

A mass transfer-based model is developed for predicting chlorine decay in drinking water distribution networks. he model considers first order reactions of chlorine to occur both in the bulk flow and at the pipe wall. he overall rate of the wall reaction is a function of the rate...

Neutron-powered precursors of kilonovae

NASA Astrophysics Data System (ADS)

Metzger, Brian D.; Bauswein, Andreas; Goriely, Stephane; Kasen, Daniel

2015-01-01

The merger of binary neutron stars (NSs) ejects a small quantity of neutron-rich matter, the radioactive decay of which powers a day to week long thermal transient known as a kilonova. Most of the ejecta remains sufficiently dense during its expansion that all neutrons are captured into nuclei during the r-process. However, recent general relativistic merger simulations by Bauswein and collaborators show that a small fraction of the ejected mass (a few per cent, or ˜10-4 M⊙) expands sufficiently rapidly for most neutrons to avoid capture. This matter originates from the shocked-heated interface between the merging NSs. Here, we show that the β-decay of these free neutrons in the outermost ejecta powers a `precursor' to the main kilonova emission, which peaks on a time-scale of ˜ few hours following merger at U-band magnitude ˜22 (for an assumed distance of 200 Mpc). The high luminosity and blue colours of the neutron precursor render it a potentially important counterpart to the gravitational wave source, that may encode valuable information on the properties of the merging binary (e.g. NS-NS versus NS-black hole) and the NS equation of state. Future work is necessary to assess the robustness of the fast-moving ejecta and the survival of free neutrons in the face of neutrino absorptions, although the precursor properties are robust to a moderate amount of leptonization. Our results provide additional motivation for short latency gravitational wave triggers and rapid follow-up searches with sensitive ground-based telescopes.

Disordered nuclear pasta, magnetic field decay, and crust cooling in neutron stars

NASA Astrophysics Data System (ADS)

Horowitz, C. J.; Berry, D. K.; Briggs, C. M.; Caplan, M. E.; Cumming, A.; Schneider, A. S.

2015-04-01

Nuclear pasta, with non-spherical shapes, is expected near the base of the crust in neutron stars. Large scale molecular dynamics simulations of pasta show long lived topological defects that could increase electron scattering and reduce both the thermal and electrical conductivities. We model a possible low conductivity pasta layer by increasing an impurity parameter Qimp. Predictions of light curves for the low mass X-ray binary MXB 1659-29, assuming a large Qimp, find continued late time cooling that is consistent with Chandra observations. The electrical and thermal conductivities are likely related. Therefore observations of late time crust cooling can provide insight on the electrical conductivity and the possible decay of neutron star magnetic fields (assuming these are supported by currents in the crust). This research was supported in part by DOE Grants DE-FG02-87ER40365 (Indiana University) and DE-SC0008808 (NUCLEI SciDAC Collaboration).

Improving the Accuracy of the Chebyshev Rational Approximation Method Using Substeps

DOE PAGES

Isotalo, Aarno; Pusa, Maria

2016-05-01

The Chebyshev Rational Approximation Method (CRAM) for solving the decay and depletion of nuclides is shown to have a remarkable decrease in error when advancing the system with the same time step and microscopic reaction rates as the previous step. This property is exploited here to achieve high accuracy in any end-of-step solution by dividing a step into equidistant sub-steps. The computational cost of identical substeps can be reduced significantly below that of an equal number of regular steps, as the LU decompositions for the linear solves required in CRAM only need to be formed on the first substep. Themore » improved accuracy provided by substeps is most relevant in decay calculations, where there have previously been concerns about the accuracy and generality of CRAM. Lastly, with substeps, CRAM can solve any decay or depletion problem with constant microscopic reaction rates to an extremely high accuracy for all nuclides with concentrations above an arbitrary limit.« less

Branching ratio of the electromagnetic decay of the Σ+(1385)

NASA Astrophysics Data System (ADS)

Keller, D.; Hicks, K.; Adhikari, K. P.; Adikaram, D.; Amaryan, M. J.; Anghinolfi, M.; Baghdasaryan, H.; Ball, J.; Battaglieri, M.; Bedlinskiy, I.; Biselli, A. S.; Bookwalter, C.; Boiarinov, S.; Branford, D.; Briscoe, W. J.; Brooks, W. K.; Burkert, V. D.; Carman, D. S.; Celentano, A.; Chandavar, S.; Cole, P. L.; Contalbrigo, M.; Crede, V.; D'Angelo, A.; Daniel, A.; Dashyan, N.; de Vita, R.; de Sanctis, E.; Djalali, C.; Doughty, D.; Dupre, R.; El Alaoui, A.; El Fassi, L.; Elouadrhiri, L.; Eugenio, P.; Fedotov, G.; Gabrielyan, M. Y.; Gevorgyan, N.; Gilfoyle, G. P.; Giovanetti, K. L.; Gohn, W.; Golovatch, E.; Gothe, R. W.; Graham, L.; Griffioen, K. A.; Guidal, M.; Guler, N.; Guo, L.; Hafidi, K.; Hakobyan, H.; Holtrop, M.; Ilieva, Y.; Ireland, D. G.; Ishkhanov, B. S.; Isupov, E. L.; Jo, H. S.; Joo, K.; Khandaker, M.; Khetarpal, P.; Kim, A.; Kim, W.; Klein, F. J.; Kubarovsky, A.; Kubarovsky, V.; Kuleshov, S. V.; Lu, H. Y.; MacGregor, I. J. D.; Mao, Y.; Markov, N.; Mayer, M.; McKinnon, B.; Meyer, C. A.; Mineeva, T.; Mirazita, M.; Mokeev, V.; Moutarde, H.; Munevar, E.; Nadel-Turonski, P.; Nasseripour, R.; Niccolai, S.; Niculescu, G.; Niculescu, I.; Osipenko, M.; Ostrovidov, A. I.; Paolone, M.; Pappalardo, L.; Paremuzyan, R.; Park, K.; Park, S.; Pasyuk, E.; Anefalos Pereira, S.; Pisano, S.; Pogorelko, O.; Pozdniakov, S.; Procureur, S.; Prok, Y.; Protopopescu, D.; Raue, B. A.; Ricco, G.; Rimal, D.; Ripani, M.; Ritchie, B. G.; Rosner, G.; Rossi, P.; Sabatié, F.; Saini, M. S.; Salgado, C.; Schott, D.; Schumacher, R. A.; Seraydaryan, H.; Sharabian, Y. G.; Smith, E. S.; Smith, G. D.; Sober, D. I.; Sokhan, D.; Stepanyan, S. S.; Stepanyan, S.; Stoler, P.; Strauch, S.; Taiuti, M.; Tang, W.; Taylor, C. E.; Tkachenko, S.; Vernarsky, B.; Vineyard, M. F.; Vlassov, A. V.; Voskanyan, H.; Voutier, E.; Watts, D. P.; Wood, M. H.; Zachariou, N.; Zana, L.; Zhao, B.; Zhao, Z. W.

2012-03-01

The CLAS detector was used to obtain the first ever measurement of the electromagnetic decay of the Σ*+(1385) from the reaction γp→K0Σ*+(1385). A real photon beam with a maximum energy of 3.8 GeV was incident on a liquid-hydrogen target, resulting in the photoproduction of the kaon and Σ* hyperon. Kinematic fitting was used to separate the reaction channel from the background processes. The fitting algorithm exploited a new method to kinematically fit neutrons in the CLAS detector, leading to the measured decay widths ratio Σ+(1385)→Σ+γ/Σ+(1385)→Σ+π0=11.95±2.21(stat)-1.21+0.53(sys)% and a deduced partial width of 250.0±56.9(stat)-41.2+34.3(sys)keV. A U-spin symmetry test using the SU(3) flavor-multiplet representation yields predictions for the Σ*+(1385)→Σ+γ and Σ*0(1385)→Λγ partial widths that agree with the experimental measurements.

Rhodium/Silver-Cocatalyzed Transannulation of N-Sulfonyl-1,2,3-triazoles with Vinyl Azides: Divergent Synthesis of Pyrroles and 2 H-Pyrazines.

PubMed

Zhang, Lin; Sun, Ge; Bi, Xihe

2016-11-07

The first cyclization reaction between vinyl azides and N-sulfonyl-1,2,3-triazoles is reported. A Rh/Ag binary metal catalyst system proved to be necessary for the successful cyclization. By varying the structure of vinyl azides, such reaction allows the divergent synthesis of pyrroles and 2H-pyrazines. The cyclization reactions feature a broad substrate scope, good functional group tolerance, high reaction efficiency, and good to high product yields. © 2016 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

RAPID COMMUNICATION: Formation of MgB2 at ambient temperature with an electrochemical process: a plausible mechanism

NASA Astrophysics Data System (ADS)

Jadhav, A. B.; Subhedar, K. M.; Hyam, R. S.; Talaptra, A.; Sen, Pintu; Bandyopadhyay, S. K.; Pawar, S. H.

2005-06-01

The binary intermetallic MgB2 superconductor has been synthesized by many research groups. However, the mechanism of its formation is not clearly understood. In this communication, a comprehensive mechanism of the formation of MgB2 from Le Chatelier's principle of equilibrium reaction has been explained both for solid-state reaction and electrodeposition methods.

Nuclear Data Sheets for A = 68

DOE Office of Scientific and Technical Information (OSTI.GOV)

McCutchan, E. A.

2012-07-01

The experimental results from the various reaction and radioactive decay studies leading to nuclides in the A = 68 mass chain have been reviewed. Nuclides ranging from Cr (Z = 24) to Br (Z = 35) are included. For these nuclei, level and decay schemes, as well as tables of nuclear properties, are given. This work supersedes the previous evaluation of the data on these nuclides (2002Bu29).

In situ arsenic oxidation and sorption by a Fe-Mn binary oxide waste in soil.

PubMed

McCann, Clare M; Peacock, Caroline L; Hudson-Edwards, Karen A; Shrimpton, Thomas; Gray, Neil D; Johnson, Karen L

2018-01-15

The ability of a Fe-Mn binary oxide waste to adsorb arsenic (As) in a historically contaminated soil was investigated. Initial laboratory sorption experiments indicated that arsenite [As(III)] was oxidized to arsenate [As(V)] by the Mn oxide component, with concurrent As(V) sorption to the Fe oxide. The binary oxide waste had As(III) and As(V) adsorption capacities of 70mgg -1 and 32mgg -1 respectively. X-ray Absorption Near-Edge Structure and Extended X-ray Absorption Fine Structure at the As K-edge confirmed that all binary oxide waste surface complexes were As(V) sorbed by mononuclear bidentate corner-sharing, with 2 Fe at ∼3.27Ǻ. The ability of the waste to perform this coupled oxidation-sorption reaction in real soils was investigated with a 10% by weight addition of the waste to an industrially As contaminated soil. Electron probe microanalysis showed As accumulation onto the Fe oxide component of the binary oxide waste, which had no As innately. The bioaccessibility of As was also significantly reduced by 7.80% (p<0.01) with binary oxide waste addition. The results indicate that Fe-Mn binary oxide wastes could provide a potential in situ remediation strategy for As and Pb immobilization in contaminated soils. Crown Copyright © 2017. Published by Elsevier B.V. All rights reserved.

Search for baryon-number and lepton-number violating decays of Λ hyperons using the CLAS detector at Jefferson Laboratory

NASA Astrophysics Data System (ADS)

McCracken, M. E.; Bellis, M.; Adhikari, K. P.; Adikaram, D.; Akbar, Z.; Pereira, S. Anefalos; Badui, R. A.; Ball, J.; Baltzell, N. A.; Battaglieri, M.; Batourine, V.; Bedlinskiy, I.; Biselli, A. S.; Boiarinov, S.; Briscoe, W. J.; Brooks, W. K.; Burkert, V. D.; Cao, T.; Carman, D. S.; Celentano, A.; Chandavar, S.; Charles, G.; Colaneri, L.; Cole, P. L.; Contalbrigo, M.; Cortes, O.; Crede, V.; D'Angelo, A.; Dashyan, N.; De Vita, R.; De Sanctis, E.; Deur, A.; Djalali, C.; Dodge, G. E.; Dupre, R.; Alaoui, A. El; Fassi, L. El; Elouadrhiri, E.; Eugenio, P.; Fedotov, G.; Fegan, S.; Fersch, R.; Filippi, A.; Fleming, J. A.; Garillon, B.; Gevorgyan, N.; Gilfoyle, G. P.; Giovanetti, K. L.; Girod, F. X.; Golovatch, E.; Gothe, R. W.; Griffioen, K. A.; Guidal, M.; Guo, L.; Hafidi, K.; Hakobyan, H.; Hanretty, C.; Hattawy, M.; Hicks, K.; Holtrop, M.; Hughes, S. M.; Ilieva, Y.; Ireland, D. G.; Ishkhanov, B. S.; Isupov, E. L.; Jenkins, D.; Jiang, H.; Jo, H. S.; Keller, D.; Khachatryan, G.; Khandaker, M.; Kim, A.; Kim, W.; Klein, A.; Klein, F. J.; Kubarovsky, V.; Lenisa, P.; Livingston, K.; Lu, H. Y.; MacGregor, I. J. D.; Mayer, M.; McKinnon, B.; Mestayer, M. D.; Meyer, C. A.; Mirazita, M.; Mokeev, V.; Moody, C. I.; Moriya, K.; Camacho, C. Munoz; Nadel-Turonski, P.; Net, L. A.; Niccolai, S.; Osipenko, M.; Ostrovidov, A. I.; Park, K.; Pasyuk, E.; Pisano, S.; Pogorelko, O.; Price, J. W.; Procureur, S.; Prok, Y.; Raue, B. A.; Ripani, M.; Rizzo, A.; Rosner, G.; Roy, P.; Sabatié, F.; Salgado, C.; Schumacher, R. A.; Seder, E.; Sharabian, Y. G.; Skorodumina, Iu.; Sokhan, D.; Sparveris, N.; Stoler, P.; Strakovsky, I. I.; Strauch, S.; Sytnik, V.; Tian, Ye; Ungaro, M.; Voskanyan, H.; Voutier, E.; Walford, N. K.; Watts, D. P.; Wei, X.; Wood, M. H.; Zachariou, N.; Zana, L.; Zhang, J.; Zhao, Z. W.; Zonta, I.; CLAS Collaboration

2015-10-01

We present a search for ten baryon number violating decay modes of Λ hyperons using the CLAS detector at Jefferson Laboratory. Nine of these decay modes result in a single meson and single lepton in the final state (Λ →m ℓ) and conserve either the sum or the difference of baryon and lepton number (B ±L ). The tenth decay mode (Λ →p ¯ π+ ) represents a difference in baryon number of two units and no difference in lepton number. We observe no significant signal and set upper limits on the branching fractions of these reactions in the range (4 - 200 )×10-7 at the 90% confidence level.

Radiative decays of the Σ0(1385) and Λ(1520) hyperons

NASA Astrophysics Data System (ADS)

Taylor, S.; Mutchler, G. S.; Adams, G.; Ambrozewicz, P.; Anciant, E.; Anghinolfi, M.; Asavapibhop, B.; Asryan, G.; Audit, G.; Avakian, H.; Bagdasaryan, H.; Ball, J. P.; Barrow, S.; Batourine, V.; Battaglieri, M.; Beard, K.; Bektasoglu, M.; Bellis, M.; Benmouna, N.; Berman, B. L.; Bianchi, N.; Biselli, A. S.; Boiarinov, S.; Bonner, B. E.; Bouchigny, S.; Bradford, R.; Branford, D.; Briscoe, W. J.; Brooks, W. K.; Bültmann, S.; Burkert, V. D.; Butuceanu, C.; Calarco, J. R.; Carman, D. S.; Carnahan, B.; Chen, S.; Cole, P. L.; Cords, D.; Corvisiero, P.; Crabb, D.; Crannell, H.; Cummings, J. P.; Sanctis, E. De; Devita, R.; Degtyarenko, P. V.; Denizli, H.; Dennis, L.; Deur, A.; Dharmawardane, K. V.; Djalali, C.; Dodge, G. E.; Doughty, D.; Dragovitsch, P.; Dugger, M.; Dytman, S.; Dzyubak, O. P.; Egiyan, H.; Egiyan, K. S.; Elouadrhiri, L.; Empl, A.; Eugenio, P.; Fatemi, R.; Feldman, G.; Fersch, R. G.; Feuerbach, R. J.; Forest, T. A.; Funsten, H.; Garçon, M.; Gavalian, G.; Gilfoyle, G. P.; Giovanetti, K. L.; Golovatch, E.; Gordon, C. I.; Gothe, R. W.; Griffioen, K. A.; Guidal, M.; Guillo, M.; Guler, N.; Guo, L.; Gyurjyan, V.; Hadjidakis, C.; Hakobyan, R. S.; Hardie, J.; Heddle, D.; Hersman, F. W.; Hicks, K.; Hleiqawi, I.; Holtrop, M.; Hu, J.; Huertas, M.; Hyde-Wright, C. E.; Ilieva, Y.; Ireland, D. G.; Ito, M. M.; Jenkins, D.; Joo, K.; Juengst, H. G.; Kellie, J. D.; Khandaker, M.; Kim, K. Y.; Kim, K.; Kim, W.; Klein, A.; Klein, F. J.; Klimenko, A. V.; Klusman, M.; Kossov, M.; Koubarovski, V.; Kramer, L. H.; Kuhn, S. E.; Kuhn, J.; Lachniet, J.; Laget, J. M.; Langheinrich, J.; Lawrence, D.; Lee, T.; Li, Ji; Lima, A. C.; Livingston, K.; Lukashin, K.; Manak, J. J.; Marchand, C.; McAleer, S.; McNabb, J. W.; Mecking, B. A.; Melone, J. J.; Mestayer, M. D.; Meyer, C. A.; Mikhailov, K.; Mirazita, M.; Miskimen, R.; Mokeev, V.; Morand, L.; Morrow, S. A.; Muccifora, V.; Mueller, J.; Napolitano, J.; Nasseripour, R.; Niccolai, S.; Niculescu, G.; Niculescu, I.; Niczyporuk, B. B.; Niyazov, R. A.; Nozar, M.; O'Rielly, G. V.; Osipenko, M.; Ostrovidov, A. I.; Park, K.; Pasyuk, E.; Philips, S. A.; Pivnyuk, N.; Pocanic, D.; Pogorelko, O.; Polli, E.; Pozdniakov, S.; Preedom, B. M.; Price, J. W.; Prok, Y.; Protopopescu, D.; Qin, L. M.; Raue, B. S.; Riccardi, G.; Ricco, G.; Ripani, M.; Ritchie, B. G.; Ronchetti, F.; Rosner, G.; Rossi, P.; Rowntree, D.; Rubin, P. D.; Sabatié, F.; Salgado, C.; Santoro, J. P.; Sapunenko, V.; Schumacher, R. A.; Serov, V. S.; Shafi, A.; Sharabian, Y. G.; Shaw, J.; Simionatto, S.; Skabelin, A. V.; Smith, E. S.; Smith, L. C.; Sober, D. I.; Spraker, M.; Stavinsky, A.; Stepanyan, S.; Stepanyan, S. S.; Stokes, B. E.; Stoler, P.; Strakovsky, I. I.; Strauch, S.; Suleiman, R.; Taiuti, M.; Tedeschi, D. J.; Thoma, U.; Thompson, R.; Tkabladze, A.; Todor, L.; Tur, C.; Ungaro, M.; Vineyard, M. F.; Vlassov, A. V.; Wang, K.; Weinstein, L. B.; Weller, H.; Weygand, D. P.; Whisnant, C. S.; Williams, M.; Wolin, E.; Wood, M. H.; Yegneswaran, A.; Yun, J.; Zana, L.

2005-05-01

The electromagnetic decays of the Σ0(1385) and Λ(1520) hyperons were studied in photon-induced reactions γp→K+Λ(1116)γ in the Large Acceptance Spectrometer detector at the Thomas Jefferson National Accelerator Facility. We report the first observation of the radiative decay of the Σ0(1385) and a measurement of the Λ(1520) radiative decay width. For the Σ0(1385)→Λ(1116)γ transition, we measured a partial width of 479±120(stat)+81-100(sys)keV, larger than all of the existing model predictions. For the Λ(1520)→Λ(1116)γ transition, we obtained a partial width of 167±43(stat)+26-12(sys)keV.

Beta-decay strength and isospin mixing studies in the sd and fp-shells

NASA Astrophysics Data System (ADS)

Jokinen, A.; ńystö, J.; Dendooven, P.; Honkanen, A.; Lipas, P.; Peräjärvi, K.; Oinonen, M.; Siiskonen, T.

1998-12-01

We have studied beta decays of MT<0 nuclei in sd and fp shells. The decay of 41Ti shows a large, 10(8) %, isospin mixing of IAS and the Gamow-Teller strength is observed to be quenched by a factor of q2=0.64. These results can be reproduced qualitatively in our shell model calculations. We have observed for the first time proton and gamma decay of the isobaric analogue state in 23Mg. Our results on the isospin mixing of the isobaric analogue state agrees well with the shell model calculations. The obtained proton branch of the IAS is used to extract the transition strength for the reaction 22Na(p,γ)23Mg.

Unstable Hadrons in Hot Hadron Gas in Laboratory and in the Early Universe

NASA Astrophysics Data System (ADS)

Kuznetsova, Inga; Rafelski, Johann

2011-04-01

We study kinetic master equations for reactions involving the formation and the natural decay of unstable particles in a thermal expanding hadronic gas in the laboratory and in the early Universe. We consider here for the first time the role of the decay channel of one (hadron resonance) into two daughter particles, and also by token of detailed balance the inverse process, fusion of two (thermal) particles into one. We obtain the thermal invariant reaction rate using as an input the free space (vacuum) decay time and show the medium quantum effects on π+π<->ρ reaction relaxation time. As another laboratory example we describe the K+K<->φ process in thermal expanding hadronic gas in heavy ions collisions. A particularly interesting application of our formalism is the 0̂<->γ+γ process in the early Universe. We also explore the fate of charged pions and the muon freeze-out in the Universe. Another interesting field of application of our formalism is the study of short lived hadronic resonances, which are in general not able to reach yield equilibrium. We study the evolution of hadron resonances in small drops of QGP and use the insight gained to generalize the dynamics to QED effects as well.

Inelastic neutron scattering cross sections for Ge 76 relevant to background in neutrinoless double- β decay experiments

DOE PAGES

Crider, B. P.; Peters, E. E.; Allmond, J. M.; ...

2015-09-11

The experimental signature in searches for the neutrinoless double- decay of 76Ge is a peak near 2039 keV in the spectrum. Given the low probability of the process, it is important that the background in this region be well understood. Moreover, inelastic scattering reactions with neutrons from muon-induced interactions and ( ,n) reactions in the surrounding materials or in the detector can provide contributions to the background. We also measured the production cross sections for rays from the 76Ge(n,n ) reaction in the 2039-keV region at incident neutron energies up to 4.9 MeV. In addition to determining that the crossmore » sections of a previously known 2040.7-keV ray from the 3952-keV level in 76 Ge are rather small, we find that a larger contribution arises from a 2037.5-keV ray which is attributed to a newly identified level at 3147 keV in 76Ge. Finally, a third contribution is also possible from another new level at 3577 keV. These results indicate that the 2039-keV region in 76Ge neutrinoless double- decay searches is more complex than was previously thought.« less

Antioxidant capacity of flavanols and gallate esters: pulse radiolysis studies.

PubMed

Bors, W; Michel, C

1999-12-01

Reactivities of several proanthocyanidins (monomers of condensed tannins) and gallate esters (representing hydrolyzable tannins) with hydroxyl radicals, azide radicals, and superoxide anions were investigated using pulse radiolysis combined with kinetic spectroscopy. We determined the scavenging rate constants and the decay kinetics of the aroxyl radicals both at the wavelength of the semiquinone absorption (275 nm) and the absorption band of the gallate ester ketyl radical (400-420 nm). For most compounds second-order decay kinetics were observed, which reflect disproportionation of the semiquinones. In the case of the oligomeric hydrolysable tannins, pentagalloyl glucose and tannic acid, the decay kinetics were more complex involving sequential first-order and second-order reactions, which could only be resolved by kinetic modeling. A correlation of the reaction rates with hydroxyl radicals (k*OH) with the number of adjacent aromatic hydroxyl groups (i.e., representing catechol and/or pyrogallol structures) was obtained for both condensed and hydrolyzable tannins. Similar correlation for the reactions with azide radicals and superoxide anions are less obvious, but exist as well. We consider proanthocyanidins superior radical scavenging agents as compared with the monomeric flavonols and flavones and propose that these substances rather than the flavonoids proper represent the antioxidative principle in red wine and green tea.

Decay of the neutron-rich isotope 171Ho and the identification of 169Dy

NASA Astrophysics Data System (ADS)

Chasteler, R. M.; Nitschke, J. M.; Firestone, R. B.; Vierinen, K. S.; Wilmarth, P. A.

1990-10-01

Neutron-rich rare-earth isotopes were produced in multinucleon transfer reactions between 170Er ions and natW targets. On-line mass separation was used together with β- and γ-ray spectroscopy in these studies. At mass A=169, the heaviest known dysprosium isotope, 39(8) s,169Dy, was identified. It was observed to β- decay to the ground state of 169Ho or through a level at 1578 keV. In the A=171 mass chain, a partial decay scheme for 55(3)-s 171Ho was determined.

The Orion Bullets: New GEMS MCAO images

NASA Astrophysics Data System (ADS)

Ginsburg, Adam; Bally, John; Youngblood, Allison

2013-07-01

The Orion A molecular cloud (OMC1) is the nearest site of massive star formation at a distance of 414 pc. The BN/KL region within it contains signs of a massive explosion triggered 500 years ago by decay of a non- hierarchical multiple system of massive stars. We present observations of the OMC1 core at high spatial resolution (<0.1") in narrow-band [Fe II] 1.64um and H2 S(1) 1-0 2.12um filters. The new data reveal compact (0.1" to 0.5") knots with unique excitation and chemical properties, unveiling new details about the three-dimensional structure of the explosion. Bright H2 emission from these compact, high proper-motion knots and compact [Fe II] features are consistent with scenario proposed by Bally et al. (2011) in which they are interpreted to be high density (n > 10^8 cm^{-3}) disk fragments launched from within a few AU of a massive star by a > three-body dynamical interaction that led to the ejection of the BN objects and the formation of a compact (separation < few AU) binary, most likely radio source I. The proper motions are as high as 400 km/s, hinting at the enormous energy unleashed in the explosion. The data also unveiled a population of obscured close binary systems. This new population will allow a comparison of embedded young binary systems with the older, un-obscured, visual binary population to test models of the evolution of multiplicity statistics in the Orion Nebula Cluster.

Merging strangeon stars

NASA Astrophysics Data System (ADS)

Lai, Xiao-Yu; Yu, Yun-Wei; Zhou, En-Ping; Li, Yun-Yang; Xu, Ren-Xin

2018-02-01

The state of supranuclear matter in compact stars remains puzzling, and it is argued that pulsars could be strangeon stars. What would happen if binary strangeon stars merge? This kind of merger could result in the formation of a hyper-massive strangeon star, accompanied by bursts of gravitational waves and electromagnetic radiation (and even a strangeon kilonova explained in the paper). The tidal polarizability of binary strangeon stars is different from that of binary neutron stars, because a strangeon star is self-bound on the surface by the fundamental strong force while a neutron star by the gravity, and their equations of state are different. Our calculation shows that the tidal polarizability of merging binary strangeon stars is favored by GW170817. Three kinds of kilonovae (i.e., of neutron, quark and strangeon) are discussed, and the light curve of the kilonova AT 2017 gfo following GW170817 could be explained by considering the decaying strangeon nuggets and remnant star spin-down. Additionally, the energy ejected to the fireball around the nascent remnant strangeon star, being manifested as a gamma-ray burst, is calculated. It is found that, after a prompt burst, an X-ray plateau could follow in a timescale of 102 ‑ 103 s. Certainly, the results could be tested also by further observational synergies between gravitational wave detectors (e.g., Advanced LIGO) and X-ray telescopes (e.g., the Chinese HXMT satellite and eXTP mission), and especially if the detected gravitational wave form is checked by peculiar equations of state provided by the numerical relativistical simulation.

Black-hole binaries as relics of gamma-ray burst/hypernova explosions

NASA Astrophysics Data System (ADS)

Moreno Mendez, Enrique

The Collapsar model, in which a fast-spinning massive star collapses into a Kerr black hole, has become the standard model to explain long-soft gamma-ray bursts and hypernova explosions (GRB/HN). However, stars massive enough (those with ZAMS mass ≳ (18--20) M⊙ ) to produce these events evolve through a path that loses too much angular momentum to produce a central engine capable of delivering the necessary energy. In this work I suggest that the soft X-ray transient sources are the remnants of GRBs/HNe. Binaries in which the massive primary star evolves a carbon-oxygen burning core, then start to transfer material to the secondary star (Case C mass transfer), causing the orbit to decay until a common-envelope phase sets in. The secondary spirals in, further narrowing the orbit of the binary and removing the hydrogen envelope of the primary star. Eventually the primary star becomes tidally locked and spins up, acquiring enough rotational energy to power up a GRB/HN explosion. The central engine producing the GRB/HN event is the Kerr black hole acting through the Blandford-Znajek mechanism. This model can explain not only the long-soft GRBs, but also the subluminous bursts (which comprise ˜ 97% of the total), the long-soft bursts and the short-hard bursts (in a neutron star, black hole merger). Because of our binary evolution through Case C mass transfer, it turns out that for the subluminous and cosmological bursts, the angular momentum O is proportional to m3/2D , where mD is the mass of the donor (secondary star). This binary evolution model has a great advantage over the Woosley Collapsar model; one can "dial" the donor mass in order to obtain whatever angular momentum is needed to drive the explosion. Population syntheses show that there are enough binaries to account for the progenitors of all known classes of GRBs.

Effect of pipe corrosion scales on chlorine dioxide consumption in drinking water distribution systems.

PubMed

Zhang, Zhe; Stout, Janet E; Yu, Victor L; Vidic, Radisav

2008-01-01

Previous studies showed that temperature and total organic carbon in drinking water would cause chlorine dioxide (ClO(2)) loss in a water distribution system and affect the efficiency of ClO(2) for Legionella control. However, among the various causes of ClO(2) loss in a drinking water distribution system, the loss of disinfectant due to the reaction with corrosion scales has not been studied in detail. In this study, the corrosion scales from a galvanized iron pipe and a copper pipe that have been in service for more than 10 years were characterized by energy dispersive spectroscopy (EDS) and X-ray diffraction (XRD). The impact of these corrosion scale materials on ClO(2) decay was investigated in de-ionized water at 25 and 45 degrees C in a batch reactor with floating glass cover. ClO(2) decay was also investigated in a specially designed reactor made from the iron and copper pipes to obtain more realistic reaction rate data. Goethite (alpha-FeOOH) and magnetite (Fe(3)O(4)) were identified as the main components of iron corrosion scale. Cuprite (Cu(2)O) was identified as the major component of copper corrosion scale. The reaction rate of ClO(2) with both iron and copper oxides followed a first-order kinetics. First-order decay rate constants for ClO(2) reactions with iron corrosion scales obtained from the used service pipe and in the iron pipe reactor itself ranged from 0.025 to 0.083 min(-1). The decay rate constant for ClO(2) with Cu(2)O powder and in the copper pipe reactor was much smaller and it ranged from 0.0052 to 0.0062 min(-1). Based on these results, it can be concluded that the corrosion scale will cause much more significant ClO(2) loss in corroded iron pipes of the distribution system than the total organic carbon that may be present in finished water.

Time-resolved production and detection of reactive atoms

DOE Office of Scientific and Technical Information (OSTI.GOV)

Grossman, L. W.; Hurst, G. S.

1977-09-01

Cesium iodide in the presence of a buffer gas was dissociated with a pulsed ultraviolet laser, which will be referred to as the source laser. This created a population of atoms at a well defined time and in a compact, well defined volume. A second pulsed laser, with a beam that completely surrounded that of the first, photoionized the cesium after a known time delay. This laser will be referred to as the detector laser. It was determined that for short time delays, all of the cesium atoms were easily ionized. When focused, the source laser generated an extremely intensemore » fluence. By accounting for the beam intensity profile it was shown that all of the molecules in the central portion of the beam can be dissociated and detected. Besides proving the feasibility of single-molecule detection, this enabled a determination of the absolute photodissociation cross section as a function of wavelength. Initial studies of the time decay of the cesium signal at low argon pressures indicated a non-exponential decay. This was consistent with a diffusion mechanism transporting cesium atoms out of the laser beam. Therefore, it was desired to conduct further experiments using a tightly focused source beam, passing along the axis of the detector beam. The theoretical behavior of this simple geometry accounting for diffusion and reaction is easily calculated. A diffusion coefficient can then be extracted by data fitting. If reactive decay is due to impurities constituting a fixed percentage of the buffer gas, then two-body reaction rates will scale linearly with pressure and three-body reaction rates will scale quadratically. Also, the diffusion coefficient will scale inversely with pressure. At low pressures it is conceivable that decay due to diffusion would be sufficiently rapid that all other processes can be neglected. Extraction of a diffusion coefficient would then be quite direct. Finally, study of the reaction of cesium and oxygen was undertaken.« less

Kinetic studies of retinol addition radicals.

PubMed

El-Agamey, Ali; Fukuzumi, Shunichi; Naqvi, K Razi; McGarvey, David J

2011-03-07

Retinol neutral radicals (RS-retinol˙), generated from the reaction of retinol with 4-pyridylthiyl and 2-pyridylthiyl radicals in argon-saturated methanol, undergo β-elimination, which can be monitored via the slow secondary absorption rise at 380 nm attributed to the rearrangement of the unstable retinol neutral addition radicals to the more stable addition radicals. Rate constants for the β-elimination reactions (k(β)) of 4-PyrS-retinol˙ were measured at different temperatures and the Arrhenius equation for the reaction is described by log (k(β)/s(-1)) = (12.7 ± 0.2) - (54.3 ± 1.3)/θ, where θ = 2.3RT kJ mol(-1). The reactivities of retinol addition radicals (RS-retinol˙), generated from the reaction of retinol with various thiyl radicals, towards oxygen have also been investigated in methanol. In the presence of oxygen, the decay of RS-retinol˙ fits to biexponential kinetics and both observed rate constants for the RS-retinol˙ decay are oxygen-concentration dependent. This suggests that at least two thiyl addition radicals, formed from the reaction of RS˙ with retinol, undergo oxygen addition reactions. In light of the estimated rate constants for oxygen addition to RS-retinol˙ and RS-CAR˙ (CAR: carotenoid), the antioxidant-prooxidant properties of retinol are discussed.

Pulse radiolytic investigations of aqueous solutions of methoxybenzene cation radicals: the effect of colloidal RuO/sub 2/

DOE Office of Scientific and Technical Information (OSTI.GOV)

Brandys, M.; Sassoon, R.E.; Rabani, J.

1987-02-12

The formation and decay of the radical cations of 1,4-dimethoxybenzene (DMB) and 1,2,4,5-tetramethoxybenzene (TMB) were investigated by the pulse radiolysis technique in the absence and the presence of colloidal RuO/sub 2/ particles. DMB/sup +/ was obtained only by Tl/sup 2 +/ oxidation of DMB while TMB/sup +/ was produced by oxidation of TMB using both Tl/sup 2 +/ and Br/sub 2//sup -/. In the absence of RuO/sub 2/ both DMB/sup +/ and TMB/sup +/ decay predominantly via a second-order process, although there is a contribution of a pseudo-first-order reaction. The rate constants for these reactions are reported. RuO/sub 2/ colloidalmore » particles catalyze the decay of both TMB/sup +/ and DMB/sup +/. The reactions of TMB/sup +/ with RuO/sub 2/ were found to depend on pH, pulse intensity, and colloid concentration. At pH 3-4, adsorption of TMB/sup +/ to the colloid is observed, followed by the decay of the remaining TMB/sup +/ in the bulk. At higher pHs, loading of the RuO/sub 2/ colloid by positive holes takes place until equilibrium is achieved between loaded holes and TMB/sup +/ and again the remaining TMB/sup +/ decays at a later stage. The fraction of TMB/sup +/ that loads the colloidal particles increases with both pH and (RuO/sub 2/). It is also suggested that DMB/sup +/ loads the RuO/sub 2/ at the pH where experiments were performed. (TMB)/sub 2/ and (DMB)/sub 2/ dimers (or higher oligomers) are suggested to be the final products both in the absence and presence of RuO/sub 2/. No O/sub 2/ is formed with the RuO/sub 2/ colloid despite a favorable redox potential for water oxidation.« less

Measurement of Neutral-Current K+ Production by Neutrinos using MINERvA

NASA Astrophysics Data System (ADS)

Marshall, C. M.; Aliaga, L.; Altinok, O.; Bellantoni, L.; Bercellie, A.; Betancourt, M.; Bodek, A.; Bravar, A.; Cai, T.; Carneiro, M. F.; da Motta, H.; Dytman, S. A.; Díaz, G. A.; Dunkman, M.; Eberly, B.; Endress, E.; Felix, J.; Fields, L.; Fine, R.; Gago, A. M.; Galindo, R.; Gallagher, H.; Ghosh, A.; Golan, T.; Gran, R.; Harris, D. A.; Higuera, A.; Hurtado, K.; Kleykamp, J.; Kordosky, M.; Le, T.; Maher, E.; Manly, S.; Mann, W. A.; Caicedo, D. A. Martinez; McFarland, K. S.; McGivern, C. L.; McGowan, A. M.; Messerly, B.; Miller, J.; Mislivec, A.; Morfín, J. G.; Mousseau, J.; Naples, D.; Nelson, J. K.; Norrick, A.; Nuruzzaman; Paolone, V.; Patrick, C. E.; Perdue, G. N.; Ramírez, M. A.; Ransome, R. D.; Ray, H.; Ren, L.; Rimal, D.; Rodrigues, P. A.; Ruterbories, D.; Schmitz, D. W.; Solano Salinas, C. J.; Sultana, M.; Sánchez Falero, S.; Valencia, E.; Walton, T.; Wolcott, J.; Wospakrik, M.; Yaeggy, B.; Zhang, D.; Minerva Collaboration

2017-07-01

Neutral-current production of K+ by atmospheric neutrinos is a background in searches for the proton decay p →K+ν ¯. Reactions such as ν p →ν K+Λ are indistinguishable from proton decays when the decay products of the Λ are below detection threshold. Events with K+ are identified in MINERvA by reconstructing the timing signature of a K+ decay at rest. A sample of 201 neutrino-induced neutral-current K+ events is used to measure differential cross sections with respect to the K+ kinetic energy, and the non-K+ hadronic visible energy. An excess of events at low hadronic visible energy is observed relative to the prediction of the neut event generator. Good agreement is observed with the cross section prediction of the genie generator. A search for photons from π0 decay, which would veto a neutral-current K+ event in a proton decay search, is performed, and a 2 σ deficit of detached photons is observed relative to the genie prediction.

Information about the 12C(α,γ)16O reaction from the β-delayed proton decay of 17Ne

NASA Astrophysics Data System (ADS)

King, J. D.; Chow, J. C.; Morton, A. C.; Azuma, R. E.; Bateman, N.; Boyd, R. N.; Buchmann, L.; D'Auria, J. M.; Davinson, T.; Dombsky, M.; Galster, W.; Gete, E.; Giesen, U.; Iliadis, C.; Jackson, K. P.; Roy, G.; Shoppa, T.; Shotter, A.

1998-02-01

We are studying the β-delayed proton decay of 17Ne with the goal of determining the E2 part of the 12C(α,γ)16O cross section at energies relevant to helium burning in stars. We have determined branching ratios for proton and α-decay for states in 17F from 8.08 to 11.193 MeV. In addition, we have observed the break-up of the isobaric analogue state (IAS) at 11.193 MeV into three particles via two channels: proton decay to the 9.59 MeV state in 16O which breaks up into an α-particle plus 12C; and α-decay to the 2.365 MeV state in 13N which breaks up into a proton plus 12C. This is the first reported observation of the decay of the IAS to the 1- state in 16O at 9.59 MeV.

Measurement of Neutral-Current K + Production by Neutrinos using MINERvA

DOE Office of Scientific and Technical Information (OSTI.GOV)

Marshall, C. M.; Aliaga, L.; Altinok, O.

Neutral-current production of K+ by atmospheric neutrinos is a background in searches for the proton decay p→K+ν¯. Reactions such as νp→νK+Λ are indistinguishable from proton decays when the decay products of the Λ are below detection threshold. Events with K+ are identified in MINERvA by reconstructing the timing signature of a K+ decay at rest. A sample of 201 neutrino-induced neutral-current K+ events is used to measure differential cross sections with respect to the K+ kinetic energy, and the non-K+ hadronic visible energy. An excess of events at low hadronic visible energy is observed relative to the prediction of themore » neut event generator. Good agreement is observed with the cross section prediction of the genie generator. A search for photons from π0 decay, which would veto a neutral-current K+ event in a proton decay search, is performed, and a 2σ deficit of detached photons is observed relative to the genie prediction.« less

W and Z boson production in p-Pb collisions at $$ \\sqrt{s_{\\mathrm{NN}}}=5.02 $$ TeV

DOE PAGES

Adam, J.; Adamová, D.; Aggarwal, M. M.; ...

2017-02-15

The W and Z boson production was measured via the muonic decay channel in proton-lead collisions at √ sNN = 5.02 TeV at the Large Hadron Collider with the ALICE detector. The measurement covers backward (–4.46 < y cms < –2.96) and forward (2.03 < y cms < 3.53) rapidity regions, corresponding to Pb-going and p-going directions, respectively. The Z-boson production cross section, with dimuon invariant mass of 60 < m μμ < 120 GeV/c 2 and muon transverse momentum (p T μ) larger than 20 GeV/c, is measured. The production cross section and charge asymmetry of muons from W-bosonmore » decays with p T μ > 10 GeV/c are determined. The results are compared to theoretical calculations both with and without including the nuclear modification of the parton distribution functions. The W-boson production is also studied as a function of the collision centrality: the cross section of muons from W-boson decays is found to scale with the average number of binary nucleon-nucleon collisions within uncertainties.« less

Simulated single molecule microscopy with SMeagol.

PubMed

Lindén, Martin; Ćurić, Vladimir; Boucharin, Alexis; Fange, David; Elf, Johan

2016-08-01

SMeagol is a software tool to simulate highly realistic microscopy data based on spatial systems biology models, in order to facilitate development, validation and optimization of advanced analysis methods for live cell single molecule microscopy data. SMeagol runs on Matlab R2014 and later, and uses compiled binaries in C for reaction-diffusion simulations. Documentation, source code and binaries for Mac OS, Windows and Ubuntu Linux can be downloaded from http://smeagol.sourceforge.net johan.elf@icm.uu.se Supplementary data are available at Bioinformatics online. © The Author 2016. Published by Oxford University Press.

Chlorine decay and trihalomethane formation following ferrate(VI) preoxidation and chlorination of drinking water.

PubMed

Li, Cong; Luo, Feng; Dong, Feilong; Zhao, Jingguo; Zhang, Tuqiao; He, Guilin; Cizmas, Leslie; Sharma, Virender K

2017-11-01

This paper presents the effect of preoxidation with ferrate(VI) (Fe VI O 4 2- , Fe(VI)) prior to chlorination on chlorine decay and formation of disinfection by-products in filtered raw water from a full-scale drinking water treatment plant. The rate of chlorine decay became significantly faster as the concentration of ferrate(VI) increased. Chlorine degradation followed two first-order decay reactions with rate constants k 1 and k 2 for fast and slow decay, respectively. Kinetic modeling established the relationships between k 1 and k 2 and varying dosages of chlorine and ferrate(VI). When ferrate(VI) was used as a pre-oxidant, the levels of trihalomethanes (trichloromethane (TCM), dichlorobromomethane (DCBM), dibromochloromethane (DBCM), and tribromomethane (TBM)) in water samples decreased as the ferrate(VI) concentration increased. The concentrations of these trihalomethanes followed the order TCM > DCBM ≈ DBCM > TBM. Copyright © 2017 Elsevier Ltd. All rights reserved.

Electron transfer from nucleophilic species to N,N,N prime ,N prime -tetramethylbenzidine cation in micellar media: Effect of interfacial electrical potential on cation decay

DOE Office of Scientific and Technical Information (OSTI.GOV)

Grand, D.; Hautecloque, S.

1990-01-25

Electron-transfer reaction between N,N,N{prime},N{prime}-tetramethylbenzidine cation (TMB{sup +}) and neutral nucleophiles, pyridine (Py) and triethylamine (Et{sub 3}N), is studied in NaLS micellar media. A biphasic decay of TMB{sup +} follows the laser-induced TMB photoionization. The very fast decay is attributed to an electron transfer between reactants located in the core of the micelle. The slow decay would correspond to an electron transfer from the nucleophile solubilized in the aqueous phase to TMB{sup +} embedded in the lipidic phase. The role of the electrical interfacial potential {Delta}{psi} is evidenced. The rate constant of the TMB{sup +} slow decay displays an exponential functionmore » of {Delta}{psi}. The effect of the localization and distance of the reactants is emphasized.« less

α decay and cluster radioactivity of nuclei of interest to the synthesis of Z =119 , 120 isotopes

NASA Astrophysics Data System (ADS)

Poenaru, D. N.; Gherghescu, R. A.

2018-04-01

Super-heavy nuclei of interest for the forthcoming synthesis of the isotopes with Z =119 , 120 are investigated. One of the very interesting latest experiments was performed at the velocity filter SHIP (GSI Darmstadt) trying to produce 299120 in a fusion reaction 248Cm(54Cr,3 n )299120 . We report calculations of α -decay half-lives using four models: AKRA (Akrawy), ASAF (analytical superasymmetric fission), UNIV (universal formula), and semFIS (semi-empirical formula based on fission theory). The released energy, Q , is calculated using the theoretical model of atomic masses, WS4. For Sr,9492 cluster radioactivity of 120,302300 we predict a branching ratio relative to α decay of -0.10 and 0.49, respectively, meaning that it is worth trying to detect such kinds of decay modes in competition with α decay.

Decay spectroscopy for nuclear astrophysics: β- and β-delayed proton decay

NASA Astrophysics Data System (ADS)

Trache, L.; Banu, A.; Hardy, J. C.; Iacob, V. E.; McCleskey, M.; Roeder, B. T.; Simmons, E.; Spiridon, A.; Tribble, R. E.; Saastamoinen, A.; Jokinen, A.; Äysto, J.; Davinson, T.; Lotay, G.; Woods, P. J.; Pollacco, E.

2012-02-01

In several radiative proton capture reactions important in novae and XRBs, the resonant parts play the capital role. We use decay spectroscopy techniques to find these resonances and study their properties. We have developed techniques to measure beta- and beta-delayed proton decay of sd-shell, proton-rich nuclei produced and separated with the MARS recoil spectrometer of Texas A&M University. The short-lived radioactive species are produced in-flight, separated, then slowed down (from about 40 MeV/u) and implanted in the middle of very thin Si detectors. This allows us to measure protons with energies as low as 200 keV from nuclei with lifetimes of 100 ms or less. At the same time we measure gamma-rays up to 8 MeV with high resolution HPGe detectors. We have studied the decay of 23Al, 27P, 31Cl, all important for understanding explosive H-burning in novae. The technique has shown a remarkable selectivity to beta-delayed charged-particle emission and works even at radioactive beam rates of a few pps. The states populated are resonances for the radiative proton capture reactions 22Na(p,γ)23Mg (crucial for the depletion of 22Na in novae), 26mAl(p,γ)27Si and 30P(p,γ)31S (bottleneck in novae and XRB burning), respectively. Lastly, results with a new detector that allowed us to measure down to about 80 keV proton energy are announced.

Fission Reaction Event Yield Algorithm

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hagmann, Christian; Verbeke, Jerome; Vogt, Ramona

FREYA (Fission Reaction Event Yield Algorithm) is a code that simulated the decay of a fissionable nucleus at specified excitation energy. In its present form, FREYA models spontaneous fission and neutron-induced fission up to 20 MeV. It includes the possibility of neutron emission from the nuclear prior to its fussion (nth chance fission).

Rate constant for the reaction SO + BrO yields SO2 + Br

NASA Technical Reports Server (NTRS)

Brunning, J.; Stief, L.

1986-01-01

The rate of the radical-radical reaction SO + BrO yields SO2 + Br has been determined at 298 K in a discharge flow system near 1 torr pressure with detection of SO and BrO via collision-free sampling mass spectrometry. The rate constant was determined using two different methods: measuring the decay of SO radicals in the presence of an excess of BrO and measuring the decay of BrO radicals in excess SO. The results from the two methods are in reasonable agreement and the simple mean of the two values gives the recommended rate constant at 298 K, k = (5.7 + or - 2.0) x 10 to the -11th cu cm/s. This represents the first determination of this rate constant and it is consistent with a previously derived lower limit based on SO2 formation. Comparison is made with other radical-radical reactions involving SO or BrO. The reaction SO + BrO yields SO2 + Br is of interest for models of the upper atmosphere of the earth and provides a potential coupling between atmospheric sulfur and bromine chemistry.

Precision measurement of the mass of the hc(1P1) state of charmonium.

PubMed

Dobbs, S; Metreveli, Z; Seth, K K; Tomaradze, A; Libby, J; Powell, A; Wilkinson, G; Ecklund, K M; Love, W; Savinov, V; Lopez, A; Mendez, H; Ramirez, J; Ge, J Y; Miller, D H; Shipsey, I P J; Xin, B; Adams, G S; Anderson, M; Cummings, J P; Danko, I; Hu, D; Moziak, B; Napolitano, J; He, Q; Insler, J; Muramatsu, H; Park, C S; Thorndike, E H; Yang, F; Artuso, M; Blusk, S; Khalil, S; Li, J; Mountain, R; Nisar, S; Randrianarivony, K; Sultana, N; Skwarnicki, T; Stone, S; Wang, J C; Zhang, L M; Bonvicini, G; Cinabro, D; Dubrovin, M; Lincoln, A; Naik, P; Rademacker, J; Asner, D M; Edwards, K W; Reed, J; Briere, R A; Ferguson, T; Tatishvili, G; Vogel, H; Watkins, M E; Rosner, J L; Alexander, J P; Cassel, D G; Duboscq, J E; Ehrlich, R; Fields, L; Galik, R S; Gibbons, L; Gray, R; Gray, S W; Hartill, D L; Heltsley, B K; Hertz, D; Hunt, J M; Kandaswamy, J; Kreinick, D L; Kuznetsov, V E; Ledoux, J; Mahlke-Krüger, H; Mohapatra, D; Onyisi, P U E; Patterson, J R; Peterson, D; Riley, D; Ryd, A; Sadoff, A J; Shi, X; Stroiney, S; Sun, W M; Wilksen, T; Athar, S B; Patel, R; Yelton, J; Rubin, P; Eisenstein, B I; Karliner, I; Mehrabyan, S; Lowrey, N; Selen, M; White, E J; Wiss, J; Mitchell, R E; Shepherd, M R; Besson, D; Pedlar, T K; Cronin-Hennessy, D; Gao, K Y; Hietala, J; Kubota, Y; Klein, T; Lang, B W; Poling, R; Scott, A W; Zweber, P

2008-10-31

A precision measurement of the mass of the h_{c}(1P1) state of charmonium has been made using a sample of 24.5x10;{6} psi(2S) events produced in e;{+}e;{-} annihilation at the Cornell Electron Storage Ring (CESR). The reaction used was psi(2S)-->pi;{0}h_{c}, pi;{0}-->gammagamma, h_{c}-->gammaeta_{c}, and the reaction products were detected in the CLEO-c detector. Data have been analyzed both for the inclusive reaction and for the exclusive reactions in which eta_{c} decays are reconstructed in 15 hadronic decay channels. Consistent results are obtained in the two analyses. The averaged results of the present measurements are M(h_{c})=3525.28+/-0.19(stat.)+/-0.12(syst.) MeV, and B(psi(2S)-->pi;{0}h_{c})xB(h_{c}-->gammaeta_{c})=(4.19+/-0.32+/-0.45)x10;{-4}. Using the ;{3}P_{J} centroid mass, DeltaM_{hf}(1P) identical withM(chi_{cJ})-M(h_{c})=+0.02+/-0.19+/-0.13 MeV.

Precision Measurement of the Mass of the hc(P11) State of Charmonium

NASA Astrophysics Data System (ADS)

Dobbs, S.; Metreveli, Z.; Seth, K. K.; Tomaradze, A.; Libby, J.; Powell, A.; Wilkinson, G.; Ecklund, K. M.; Love, W.; Savinov, V.; Lopez, A.; Mendez, H.; Ramirez, J.; Ge, J. Y.; Miller, D. H.; Shipsey, I. P. J.; Xin, B.; Adams, G. S.; Anderson, M.; Cummings, J. P.; Danko, I.; Hu, D.; Moziak, B.; Napolitano, J.; He, Q.; Insler, J.; Muramatsu, H.; Park, C. S.; Thorndike, E. H.; Yang, F.; Artuso, M.; Blusk, S.; Khalil, S.; Li, J.; Mountain, R.; Nisar, S.; Randrianarivony, K.; Sultana, N.; Skwarnicki, T.; Stone, S.; Wang, J. C.; Zhang, L. M.; Bonvicini, G.; Cinabro, D.; Dubrovin, M.; Lincoln, A.; Naik, P.; Rademacker, J.; Asner, D. M.; Edwards, K. W.; Reed, J.; Briere, R. A.; Ferguson, T.; Tatishvili, G.; Vogel, H.; Watkins, M. E.; Rosner, J. L.; Alexander, J. P.; Cassel, D. G.; Duboscq, J. E.; Ehrlich, R.; Fields, L.; Galik, R. S.; Gibbons, L.; Gray, R.; Gray, S. W.; Hartill, D. L.; Heltsley, B. K.; Hertz, D.; Hunt, J. M.; Kandaswamy, J.; Kreinick, D. L.; Kuznetsov, V. E.; Ledoux, J.; Mahlke-Krüger, H.; Mohapatra, D.; Onyisi, P. U. E.; Patterson, J. R.; Peterson, D.; Riley, D.; Ryd, A.; Sadoff, A. J.; Shi, X.; Stroiney, S.; Sun, W. M.; Wilksen, T.; Athar, S. B.; Patel, R.; Yelton, J.; Rubin, P.; Eisenstein, B. I.; Karliner, I.; Mehrabyan, S.; Lowrey, N.; Selen, M.; White, E. J.; Wiss, J.; Mitchell, R. E.; Shepherd, M. R.; Besson, D.; Pedlar, T. K.; Cronin-Hennessy, D.; Gao, K. Y.; Hietala, J.; Kubota, Y.; Klein, T.; Lang, B. W.; Poling, R.; Scott, A. W.; Zweber, P.

2008-10-01

A precision measurement of the mass of the hc(P11) state of charmonium has been made using a sample of 24.5×106 ψ(2S) events produced in e+e- annihilation at the Cornell Electron Storage Ring (CESR). The reaction used was ψ(2S)→π0hc, π0→γγ, hc→γηc, and the reaction products were detected in the CLEO-c detector. Data have been analyzed both for the inclusive reaction and for the exclusive reactions in which ηc decays are reconstructed in 15 hadronic decay channels. Consistent results are obtained in the two analyses. The averaged results of the present measurements are M(hc)=3525.28±0.19(stat.)±0.12(syst.)MeV, and B(ψ(2S)→π0hc)×B(hc→γηc)=(4.19±0.32±0.45)×10-4. Using the PJ3 centroid mass, ΔMhf(1P)≡⟨M(χcJ)⟩-M(hc)=+0.02±0.19±0.13MeV.

The Syntheses and Structure of the First Vanadium(IV) and Vanadium(V) Binary Azides, V(N3)4, [V(N3)6]2- and [V(N3)6]- (Preprint)

DTIC Science & Technology

2009-11-17

V(N3)3(N3S2)] 2- , [22] have been reported, and no binary vanadium(V) compounds had been known except for VF5, VF6 - and V2O5 . By analogy with...valves. Volatile materials were handled in a Pyrex glass or stainless steel/Teflon-FEP vacuum line. [31] All reaction vessels were passivated with ClF3...successful synthesis of the [V(N3)6] - anion, the only binary vanadium(V) compound known besides VF5, VF6 - and V2O5 . N1’ N8 N9 N1 N2 N3 V N4 N5 N6 N2

Interrogation of bimetallic particle oxidation in three dimensions at the nanoscale

DOE PAGES

Han, Lili; Meng, Qingping; Wang, Deli; ...

2016-12-08

An understanding of bimetallic alloy oxidation is key to the design of hollow-structured binary oxides and the optimization of their catalytic performance. However, one roadblock encountered in studying these binary oxide systems is the difficulty in describing the heterogeneities that occur in both structure and chemistry as a function of reaction coordinate. This is due to the complexity of the three-dimensional mosaic patterns that occur in these heterogeneous binary systems. By combining real-time imaging and chemical-sensitive electron tomography, we show that it is possible to characterize these systems with simultaneous nanoscale and chemical detail. We find that there is oxidation-inducedmore » chemical segregation occurring on both external and internal surfaces. Additionally, there is another layer of complexity that occurs during the oxidation, namely that the morphology of the initial oxide surface can change the oxidation modality. As a result, this work characterizes the pathways that can control the morphology in binary oxide materials.« less

Development of a Portable Binary Chlorine Dioxide Generator for Decontamination

DTIC Science & Technology

2010-03-01

chlorine dioxide forms slowly from chlorite solutions through either acid release or a radical chain reaction that we observed at neutral pH. Task 7... Chlorine dioxide and water in methanol - no agent control F. 5.25% Bleach G. Methanol only 3.0 PROCEDURES 3.1 METHOD VALIDATION The reaction...error range in gas chromatography measurements. For the chlorine dioxide containing samples, mass spectra were analyzed to determine potential

Nuclear Data Sheets for A = 69

NASA Astrophysics Data System (ADS)

Nesaraja, C. D.

2014-01-01

Experimental data on ground- and excited-state properties for all known nuclei with mass number A = 69 have been compiled and evaluated. States populated in radioactive decay, as well as in nuclear reactions, have been considered. For these nuclei, level and decay schemes, as well as tables of nuclear properties, are given in detail. This work supersedes the 2000 evaluation by M.R. Bhat and J.K. Tuli (2000Bh05).

Nuclear Data Sheets for A=69

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nesaraja, C.D.

Experimental data on ground– and excited–state properties for all known nuclei with mass number A=69 have been compiled and evaluated. States populated in radioactive decay, as well as in nuclear reactions, have been considered. For these nuclei, level and decay schemes, as well as tables of nuclear properties, are given in detail. This work supersedes the 2000 evaluation by M.R. Bhat and J.K. Tuli (2000Bh05)

Recombination of H(3+) and D(3+) ions with electrons

NASA Technical Reports Server (NTRS)

Johnsen, R.; Gougousi, T.; Golde, M. F.

1994-01-01

Flowing-afterglow measurements in decaying H3(+) or D3(+) plasmas suggest that de-ionization does not occur by simple binary recombination of a single ion species. We find that vibrational excitation of the ions fails to provide an explanation for the effect, contrary to an earlier suggestion. Instead, we suggest that collisional stabilization of H3** Rydberg molecules by ambient electrons introduces an additional dependence on electron density. The proposed mechanism would permit plasma de-ionization to occur without the need for dissociative recombination by the mechanism of potential-surface crossings.

Unimolecular reaction of acetone oxide and its reaction with water in the atmosphere.

PubMed

Long, Bo; Bao, Junwei Lucas; Truhlar, Donald G

2018-05-29

Criegee intermediates (i.e., carbonyl oxides with two radical sites) are known to be important atmospheric reagents; however, our knowledge of their reaction kinetics is still limited. Although experimental methods have been developed to directly measure the reaction rate constants of stabilized Criegee intermediates, the experimental results cover limited temperature ranges and do not completely agree well with one another. Here we investigate the unimolecular reaction of acetone oxide [(CH 3 ) 2 COO] and its bimolecular reaction with H 2 O to obtain rate constants with quantitative accuracy comparable to experimental accuracy. We do this by using CCSDT(Q)/CBS//CCSD(T)-F12a/DZ-F12 benchmark results to select and validate exchange-correlation functionals, which are then used for direct dynamics calculations by variational transition state theory with small-curvature tunneling and torsional and high-frequency anharmonicity. We find that tunneling is very significant in the unimolecular reaction of (CH 3 ) 2 COO and its bimolecular reaction with H 2 O. We show that the atmospheric lifetimes of (CH 3 ) 2 COO depend on temperature and that the unimolecular reaction of (CH 3 ) 2 COO is the dominant decay mode above 240 K, while the (CH 3 ) 2 COO + SO 2 reaction can compete with the corresponding unimolecular reaction below 240 K when the SO 2 concentration is 9 × 10 10 molecules per cubic centimeter. We also find that experimental results may not be sufficiently accurate for the unimolecular reaction of (CH 3 ) 2 COO above 310 K. Not only does the present investigation provide insights into the decay of (CH 3 ) 2 COO in the atmosphere, but it also provides an illustration of how to use theoretical methods to predict quantitative rate constants of medium-sized Criegee intermediates.

The Gaseous Explosive Reaction : the Effect of Pressure on the Rate of Propagation of the Reaction Zone and upon the Rate of Molecular Transformation

NASA Technical Reports Server (NTRS)

Stevens, F W

1932-01-01

This study of gaseous explosive reaction has brought out a number of important fundamental characteristics of the explosive reaction indicating that the basal processes of the transformation are much simpler and corresponds more closely to the general laws and principles of ordinary transformations than is usually supposed. The report calls attention to the point that the rate of molecular transformation within the zone was found in all cases to be proportional to pressure, that the transformation within the zone is the result of binary impacts. This result is of unusual interest in the case of the reaction of heavy hydrocarbon fuels and the reaction mechanism proposed by the recent kinetic theory of chain reactions.

Correlation of gravestone decay and air quality 1960-2010

NASA Astrophysics Data System (ADS)

Mooers, H. D.; Carlson, M. J.; Harrison, R. M.; Inkpen, R. J.; Loeffler, S.

2017-03-01

Evaluation of spatial and temporal variability in surface recession of lead-lettered Carrara marble gravestones provides a quantitative measure of acid flux to the stone surfaces and is closely related to local land use and air quality. Correlation of stone decay, land use, and air quality for the period after 1960 when reliable estimates of atmospheric pollution are available is evaluated. Gravestone decay and SO2 measurements are interpolated spatially using deterministic and geostatistical techniques. A general lack of spatial correlation was identified and therefore a land-use-based technique for correlation of stone decay and air quality is employed. Decadally averaged stone decay is highly correlated with land use averaged spatially over an optimum radius of ≈7 km even though air quality, determined by records from the UK monitoring network, is not highly correlated with gravestone decay. The relationships among stone decay, air-quality, and land use is complicated by the relatively low spatial density of both gravestone decay and air quality data and the fact that air quality data is available only as annual averages and therefore seasonal dependence cannot be evaluated. However, acid deposition calculated from gravestone decay suggests that the deposition efficiency of SO2 has increased appreciably since 1980 indicating an increase in the SO2 oxidation process possibly related to reactions with ammonia.

Results from the First {sup 249}Cf + {sup 48}Ca Experiment

DOE R&D Accomplishments Database

Oganessian, Y. T.; Utyonkov, V. K.; Lobanov, Y. V.; Abdullin, F. S.; Polyakov, A. N.; Shirokovsky, I. V.; Tsyganov, Y. S.; Mezentsev, A. N.; Iliev, S.; Subbotin, V. G.; Sukhov, A. M.; Ivanov, O. V.; Voinov, A. A.; Subotic, K.; Zagrebaev, V. I.; Itkis, M. G.; Moody, K. J.; Wild, J. F.; Stoyer, M. A.; Stoyer, N. J.; Laue, C. A.; Shaughnessy, D. A.; Patin, J. B.; Lougheed, R. W.

2003-02-03

The present paper reports the results of an attempt aimed at the synthesis of element 118 in the reaction {sup 249}Cf({sup 48}Ca,3n){sup 294}118. The experiment was performed employing the Dubna Gas-filled Recoil Separator and the U400 heavy-ion cyclotron at FLNR, JINR, Dubna. In the course of a 2300-hour irradiation of an enriched {sup 249}Cf target (0.23 mg/cm{sup 2}) with a beam of 245-MeV {sup 48}Ca ions, we accumulated a total beam dose of 2.5 x 10{sup 19} ions. We detected two events that may be attributed to the formation and decay of nuclei with Z=118. For one event, we observed a decay chain of two correlated {alpha}-decays with corresponding energies and correlation times of E{sub {alpha}1} = 11.65 {+-} 0.06 MeV, t{sub {alpha}1} = 2.55 ms and E{sub {alpha}2} = 10.71 {+-} 0.17 MeV, t{sub {alpha}2} = 42.1 ms and, finally, a spontaneous fission with the sum of the kinetic energies of the fission fragments E{sub tot} = 207 MeV (TKE {approx} 230 MeV) and t{sub SF} = 0.52 s. In the second event chain, the recoil nucleus decayed into two fission fragments with E{sub tot} = 223 MeV (TKE {approx} 245 MeV) 3.16 ms later, without intervening {alpha} decays. The probabilities that these events were caused by the chance correlations of unrelated signals are negligible. Both events were observed at an excitation energy of the compound nucleus {sup 297}118 of E* = 30.0 {+-} 2.4 MeV, close to the expected maximum of the 3n-evaporation channel. The relationship between the decay energy Q{sub {alpha}} and decay period T{sub {alpha}} shows that sequential {alpha}-transitions in the first event correspond to the decay chain with Z = 118{_}116{_}114. Decay characteristics of the newly observed nuclides are compared with radioactive decay properties of the even-even isotopes with Z = 116, 114 and 112 previously produced in the reactions {sup 244}Pu, {sup 248}Cm + {sup 48}Ca and calculations made in various nuclear models.

Synthesis of nonionic-anionic colloidal systems based on alkaline and ammonium β-nonylphenol polyethyleneoxy (n = 3-20) propionates/dodecylbenzenesulfonates with prospects for food hygiene

PubMed Central

2012-01-01

Background The main objective of this work was to obtain a binary system of surface-active components (nonionic soap – alkaline and/or ammonium dodecylbenzenesulfonate) with potential competences in food hygiene, by accessing a scheme of classical reactions (cyanoethylation, total acid hydrolysis and stoichiometric neutralization with inorganic alkaline and/or organic ammonium bases) adapted to heterogeneously polyethoxylated nonylphenols (n = 3-20). In the processing system mentioned, dodecylbenzenesulfonic acid, initially the acid catalyst for the exhaustive hydrolysis of β-nonylphenolpolyethyleneoxy (n = 3-20) propionitriles, becomes together with the nonionic soap formed the second surface-active component of the binary system. Results In the reaction scheme adopted the influence of the main operating (duration, temperature, molar ratio of reagents) and structural parameters (degree of oligomerization of the polyoxyethylene chain) on the processing yields for the synthetic steps was followed. The favorable role of the polyoxyethylene chain size is remarked, through its specific conformation and its alkaline cations sequestration competences on the yields of cyanoethylation, but also the beneficial influence of phase-transfer catalysts in the total acid hydrolysis step. The chemical stability of dodecylbenzenesulfonic acid (DBSH) at the temperature and strongly acidic pH of the reaction environment is confirmed. The controlled change of the amount of DBSH in the final binary system will later confer it potential colloidal competences in food hygiene receipts. Conclusions The preliminary synthetic tests performed confirmed the prospect of obtaining a broad range of useful colloidal competences in various food hygiene scenarios. PMID:22958389

The Neutron Star Zoo

NASA Technical Reports Server (NTRS)

Harding, Alice K.

2014-01-01

Neutron stars are a very diverse population, both in their observational and their physical properties. They prefer to radiate most of their energy at X-ray and gamma-ray wavelengths. But whether their emission is powered by rotation, accretion, heat, magnetic fields or nuclear reactions, they are all different species of the same animal whose magnetic field evolution and interior composition remain a mystery. This article will broadly review the properties of inhabitants of the neutron star zoo, with emphasis on their high-energy emission. XXX Neutron stars are found in a wide variety of sources, displaying an amazing array of behavior. They can be isolated or in binary systems, accreting, heating, cooling, spinning down, spinning up, pulsing, flaring and bursting. The one property that seems to determine their behavior most strongly is their magnetic field strength, structure and evolution. The hot polar caps, bursts and flares of magnetars are likely due to the rapid decay and twisting of their superstrong magnetic fields, whose very existence requires some kind of early dynamo activity. The intermediate-strength magnetic fields of RPPs determines their spin-down behavior and radiation properties. However, the overlap of the magnetar and RPP populations is not understood at present. Why don't high-field RPPs burst or flare? Why don't lower-field magnetars sometimes behave more like RPPs? INS may be old magnetars whose high fields have decayed, but they do not account for the existence of younger RPPs with magnetar-strength fields. Not only the strength of the magnetic field but also its configuration may be important in making a NS a magnetar or a RPP. Magnetic field decay is a critical link between other NS populations as well. "Decay" of the magnetic field is necessary for normal RPPs to evolve into MSPs through accretion and spin up in LMXBs. Some kind of accretion-driven field reduction is the most likely mechanism, but it is controversial since it is not clear how effective it is or on what timescale a buried field might re-emerge. One piece of evidence in favor of accretion-driven field reduction is the fact that NSs in LMXBs, which are older systems (> 108 yr), have mostly low fields and NSs in HMXBs, which are younger systems (107 - 108 yr), have higher fields. This may be an indication that accretion-driven field reduction or decay has not had enough time to operate in HMXBs but has in LMXBs. However, there does not seem to be any evidence of decaying fields in either the LMXB or HMXB populations; e.g. smaller magnetic fields in older systems. On the other hand, CCOs are very young so if they acquired their low fields through mass fallback accretion, the field submergence would have had to operate on much faster timescales than it apparently does in LMXBs. But as we continue to find new species in the NS zoo, one of these may someday be the "Rosetta Stone" that will give us the clues for solving these puzzles.

Nitric oxide density measurements in air and air/fuel nanosecond pulse discharges by laser induced fluorescence

NASA Astrophysics Data System (ADS)

Uddi, M.; Jiang, N.; Adamovich, I. V.; Lempert, W. R.

2009-04-01

Laser induced fluorescence is used to measure absolute nitric oxide concentrations in air, methane-air and ethylene-air non-equilibrium plasmas, as a function of time after initiation of a single pulse, 20 kV peak voltage, 25 ns pulse duration discharge. A mixture of NO and nitrogen with known composition (4.18 ppm NO) is used for calibration. Peak NO density in air at 60 Torr, after a single pulse, is ~8 × 1012 cm-3 (~4.14 ppm) occurring at ~250 µs after the pulse, with decay time of ~16.5 ms. Peak NO atom mole fraction in a methane-air mixture with equivalence ratio of phiv = 0.5 is found to be approximately equal to that in air, with approximately the same rise and decay rate. In an ethylene-air mixture (also with equivalence ratio of phiv = 0.5), the rise and decay times are comparable to air and methane-air, but the peak NO concentration is reduced by a factor of approximately 2.5. Spontaneous emission measurements show that excited electronic states N2(C 3Π) and NO(A 2Σ) in air at P = 60 Torr decay within ~20 ns and ~1 µs, respectively. Kinetic modelling calculations incorporating air plasma kinetics complemented with the GRI Mech 3.0 hydrocarbon oxidation mechanism are compared with the experimental data using three different NO production mechanisms. It is found that NO concentration rise after the discharge pulse is much faster than predicted by Zel'dovich mechanism reactions, by two orders of magnitude, but much slower compared with reactions of electronically excited nitrogen atoms and molecules, also by two orders of magnitude. It is concluded that processes involving long lifetime (~100 µs) metastable states, such as N2(X 1Σ,v) and O2(b 1Σ), formed by quenching of the metastable N2(A 3Σ) state by ground electronic state O2, may play a dominant role in NO formation. NO decay, in all cases, is found to be dominated by the reverse Zel'dovich reaction, NO + O → N + O2, as well as by conversion into NO2 in a reaction of NO with ozone.

Search for baryon-number and lepton-number violating decays of Λ hyperons using the CLAS detector at Jefferson Laboratory

DOE PAGES

McCracken, Michael E.

2015-10-09

We present a search for ten baryon-number violating decay modes of Λ hyperons using the CLAS detector at Jefferson Laboratory. Nine of these decay modes result in a single meson and single lepton in the final state (Λ → mΙ) and conserve either the sum or the difference of baryon and lepton number (Β ± L). The tenth decay mode (Λ → p¯π +) represents a difference in baryon number of two units and no difference in lepton number. Furthermore, we observe no significant signal and set upper limits on the branching fractions of these reactions in the range (4more » – 200) x 10 7 at the 90% confidence level.« less

Mass correlation between light and heavy reaction products in multinucleon transfer 197Au+130Te collisions

NASA Astrophysics Data System (ADS)

Galtarossa, F.; Corradi, L.; Szilner, S.; Fioretto, E.; Pollarolo, G.; Mijatović, T.; Montanari, D.; Ackermann, D.; Bourgin, D.; Courtin, S.; Fruet, G.; Goasduff, A.; Grebosz, J.; Haas, F.; Jelavić Malenica, D.; Jeong, S. C.; Jia, H. M.; John, P. R.; Mengoni, D.; Milin, M.; Montagnoli, G.; Scarlassara, F.; Skukan, N.; Soić, N.; Stefanini, A. M.; Strano, E.; Tokić, V.; Ur, C. A.; Valiente-Dobón, J. J.; Watanabe, Y. X.

2018-05-01

We studied multinucleon transfer reactions in the 197Au+130Te system at Elab=1.07 GeV by employing the PRISMA magnetic spectrometer coupled to a coincident detector. For each light fragment we constructed, in coincidence, the distribution in mass of the heavy partner of the reaction. With a Monte Carlo method, starting from the binary character of the reaction, we simulated the de-excitation process of the produced heavy fragments to be able to understand their final mass distribution. The total cross sections for pure neutron transfer channels have also been extracted and compared with calculations performed with the grazing code.

Photoinduced Reactions of Benzophenone in Biaxially Oriented Polypropylene.

PubMed

Levin, Peter P; Efremkin, Alexei F; Krivandin, Aleksey V; Lomakin, Sergei M; Shatalova, Olga V; Khudyakov, Igor V

2018-05-03

The photoinduced reactions of benzophenone (B) in biaxially oriented polypropylene (BOPP) were studied with nanosecond laser photolysis (N 2 laser, λ337.1 nm). The first observed transient was a triplet state 3 B*. Decay of 3 B* led to formation of a radical pair (RP) of BH • and R • , where R • is a radical formed by hydrogen abstraction from BOPP (RH) by 3 B*. We studied BOPP after the preheating for a short time in a temperature range 298-423 K, which is essentially lower than its melting point of 453 K. All measurements with not-heated and with preheated (annealed) BOPP were made at 298 K. A radical pair (RP) apparently decays as a contact pair 3 [BH • , R • ] in nonheated BOPP. A critical phenomenon takes place: dissociation of RP with a formation of free radicals in the polymer bulk is observed at preheating temperature T crit ≈ 403 K and at a higher T. The physical process of heating and cooling of BOPP apparently resulted in the restructuring of crystallites, their agglomeration, shrinking of the distribution of crystallites according to their sizes in BOPP. Overall BOPP becomes softer which manifests itself in the radical kinetics. The decay kinetics of 3 B* and RP in the cage fits well the first-order law. Rate constants were obtained. Radicals BH • , which exit into the polymer bulk at temperatures of preheating T ≥ 403 K, decay by cross-termination according to the second-order law. A relatively high rate constant ∼10 8 M -1 ·s -1 for this reaction was obtained due to diffusion of BH • enclosed in the soft amorphous phase of BOPP. Properties of BOPP containing B were studied with ESR, DSC, IR, and WAXD.

Photonuclear reactions triggered by lightning discharge.

PubMed

Enoto, Teruaki; Wada, Yuuki; Furuta, Yoshihiro; Nakazawa, Kazuhiro; Yuasa, Takayuki; Okuda, Kazufumi; Makishima, Kazuo; Sato, Mitsuteru; Sato, Yousuke; Nakano, Toshio; Umemoto, Daigo; Tsuchiya, Harufumi

2017-11-22

Lightning and thunderclouds are natural particle accelerators. Avalanches of relativistic runaway electrons, which develop in electric fields within thunderclouds, emit bremsstrahlung γ-rays. These γ-rays have been detected by ground-based observatories, by airborne detectors and as terrestrial γ-ray flashes from space. The energy of the γ-rays is sufficiently high that they can trigger atmospheric photonuclear reactions that produce neutrons and eventually positrons via β + decay of the unstable radioactive isotopes, most notably 13 N, which is generated via 14 N + γ →  13 N + n, where γ denotes a photon and n a neutron. However, this reaction has hitherto not been observed conclusively, despite increasing observational evidence of neutrons and positrons that are presumably derived from such reactions. Here we report ground-based observations of neutron and positron signals after lightning. During a thunderstorm on 6 February 2017 in Japan, a γ-ray flash with a duration of less than one millisecond was detected at our monitoring sites 0.5-1.7 kilometres away from the lightning. The subsequent γ-ray afterglow subsided quickly, with an exponential decay constant of 40-60 milliseconds, and was followed by prolonged line emission at about 0.511 megaelectronvolts, which lasted for a minute. The observed decay timescale and spectral cutoff at about 10 megaelectronvolts of the γ-ray afterglow are well explained by de-excitation γ-rays from nuclei excited by neutron capture. The centre energy of the prolonged line emission corresponds to electron-positron annihilation, providing conclusive evidence of positrons being produced after the lightning.

Nuclear structure studies in the seaborgium region at SHIP

DOE Office of Scientific and Technical Information (OSTI.GOV)

Antalic, S., E-mail: Stanislav.Antalic@fmph.uniba.sk; Andel, B.; Heßberger, F. P.

2015-10-15

New decay data for the isotopes {sup 259}Sg and {sup 255}Rf were obtained at the velocity filter SHIP using an α-decay spectroscopy measurement. Both isotopes were produced and studied via a one neutron evaporation channel in the compound fusion reaction {sup 54}Cr+{sup 208}Pb. New isomeric states were observed and the single-particle level systematics for isotones with 151 and 153 neutrons were extended. A change of the ground-state configuration for the heaviest N = 151 isotones was observed. Detailed Monte-Carlo simulation for the α decay of {sup 259}Sg applying the GEANT4 toolkit was performed and compared with experimental data.

Nuclear Data Sheets for A = 138

NASA Astrophysics Data System (ADS)

Sonzogni, A. A.

2003-03-01

Experimental data on ground- and excited-state properties for all known nuclei with mass number A=138 have been compiled and evaluated. States populated in radioactive decay as well as in nuclear reactions have been considered. For these nuclei, level and decay schemes, as well as tables of nuclear properties are given. This work supersedes the 1995 evaluation by J.K. Tuli (1995Tu01). Manuscripts published before December 2002 have been included in this work.

2-Hydroxypropyltrimethylammonium xylan adsorption onto rod-like cellulose nanocrystal.

PubMed

Sim, Jae Hyun; Dong, Shuping; Röemhild, Katrin; Kaya, Abdulaziz; Sohn, Daewon; Tanaka, Keiji; Roman, Maren; Heinze, Thomas; Esker, Alan R

2015-02-15

Chemical incompatibility and relatively weak interaction between lignocellulosic fibers and synthetic polymers have made studies of wood fiber-thermoplastic composite more challenging. In this study, adsorption of 2-hydroxypropyltrimethylammonium xylans onto rod-like cellulose nanocrystals are investigated by zeta-potential measurements, and polarized and depolarized dynamic light scattering as a factor for better understanding of lignocellulosic fibers and cellulose nanocrystals. Zeta-potential measurements show xylan derivative adsorption onto cellulose nanocrystals. Decay time distributions of the ternary system and binary system from dynamic light scattering show that aggregates exist in the binary system and they disappear in the ternary system. At low 2-hydroxypropyltrimethylammonium xylan concentrations relative to that of cellulose nanocrystal, xylan derivatives adsorbed onto some of the cellulose nanocrystal. Hence, more xylan derivatives adsorbed onto cellulose nanocrystal increased with increasing xylan derivative concentration. Also, the concentration dependence of the ratio of the rotational diffusion coefficient to the translational diffusion coefficient revealed a strong adsorptive interaction between xylan derivatives and the cellulose nanocrystals. Copyright © 2014 Elsevier Inc. All rights reserved.

X-RAY SOURCES IN THE DWARF SPHEROIDAL GALAXY DRACO

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sonbas, E.; Rangelov, B.; Kargaltsev, O.

2016-04-10

We present the spectral analysis of an 87 ks XMM-Newton observation of Draco, a nearby dwarf spheroidal galaxy. Of the approximately 35 robust X-ray source detections, we focus our attention on the brightest of these sources, for which we report X-ray and multiwavelength parameters. While most of the sources exhibit properties consistent with active galactic nuclei, few of them possess the characteristics of low-mass X-ray binaries (LMXBs) and cataclysmic variable (CVs). Our analysis places constraints on the population of X-ray sources with L{sub X} > 3 × 10{sup 33} erg s{sup −1} in Draco, suggesting that there are no actively accreting black hole andmore » neutron star binaries. However, we find four sources that could be quiescent state LMXBs/CVs associated with Draco. We also place constraints on the central black hole luminosity and on a dark matter decay signal around 3.5 keV.« less

The MXB1916-053/4U1915-05: Burst properties and constraints on a 50 minute binary secondary

NASA Technical Reports Server (NTRS)

Swank, J. H.; Taam, R. E.; White, N. E.

1983-01-01

Results are presented from OSO-8 and HEAO-1 A2 observations of 34 bursts from the X-ray burster MXB1916-053/4U1915-05 recently discovered to show a 50 minute binary period. While 11 burst previously reported all had similar light curves, 22 observed two years later show a factor of 3 range of peak fluxes and decay times between 3 and 20 s. Recurrence times between successive bursts vary between 3 and 6 hours. A ratio of steady flux to average burst flux of equiv 120 is developed. A burst observed with the HEAO-1 A2 experiment showed an initial temperature rise to a peak black body temperature of equiv 3 keV followed by the cooling typical of type I bursts. The burst was unusual in that the apparent projected size of a blackbody source increased by a factor of 3 during the cooling phase.

Ginga observations of the dipping low-mass X-ray binaries XB 1916-053 and EXO 1748-676

NASA Technical Reports Server (NTRS)

Smale, Alan P.; Mukai, Koji; Williams, O. R.; Jones, Mark H.; Corbet, Robin H. D.

1992-01-01

Ginga observations of XB 1916-053 and EXO 0748-676, low-mass X-ray binaries with pronounced dips of variable depth and duration in their X-ray light curves, are reported. Periodicity studies of XB-1916-053 show results consistent with those from previous Ginga observations, specifically, that the derived X-ray period is shorter than the optical period by about 1 percent. This problem is discussed, and a more refined model for the system is described. Three bursts were detected during the observation of XB 1916-053, the second of which occurred during a dip. Spectral analysis suggests that the second burst caused an almost instantaneous ionization of the absorbing medium in the line of sight. This material then returned to its equilibrium state on the same time scale as the burst decay. Loose limits are placed upon the possible clumpiness of the material responsible for the accretion disk structure in XB 1916-053 and EXO 0748-676.

The Feasibility of Studying 44Ti(α, p)47V Reaction at Astrophysical Energies

NASA Astrophysics Data System (ADS)

Al-Abdullah, Tariq; Bemmerer, D.; Elekes, Z.; Schumann, D.

2018-01-01

The gamma-ray lines from the decay of 44Ti have been observed by space-based gamma-ray telescopes from two supernova remnants. It is believed that the 44Ti(α, p)47V reaction dominates the destruction of 44Ti. This work presents a possible technique to determine its reaction rate in forward kinematics at astrophysically relevant energies. Several online and offline measurements in parallel with Monte Carlo simulations were performed to illustrate the feasibility of performing this reaction. The results will be discussed.

Relative role of different radii in the dynamics of 8B+58Ni reaction

NASA Astrophysics Data System (ADS)

Kaur, Amandeep; Sandhu, Kirandeep; Sharma, Manoj K.

2018-05-01

In the present work, we intend to analyze the significance of three different radius terms in the framework of dynamical cluster-decay model (DCM) based calculations. In the majority of DCM based calculations the impact of mass- dependent radius R(A) is extensively analyzed. The other two factors on which the radius term may depend are, the neutron- proton asymmetry and the charge of the decaying fragments. Hence, the asymmetry dependent radius term R(I) and charge dependent radius term R(Z) are incorporated in DCM based calculations to investigate their effect on the reaction dynamics involved. Here, we present an extension of an earlier work based on the decay of 66As* compound nucleus by including R(I) and R(Z) radii in addition to the R(A) term. The effect of replacement of R(A) with R(I) and R(Z) is analyzed via fragmentation structure, tunneling probabilities (P) and other barrier characteristics like barrier height (VB), barrier position (RB), barrier turning point Ra etc. The role of temperature, deformations and angular momentum is duly incorporated in the present calculations.

Photodegradation mechanism and rate improvement of chlorinated aromatic dye in non-ionic surfactant solutions.

PubMed

Ma, C W; Chu, W

2001-07-01

A typical insoluble chlorinated aromatic dye (CAD), disperse red (DR), was used to explore the reaction mechanism and kinetics of photodegradation in non-ionic surfactant solutions. The use of an additional hydrogen source and photosensitizer is also studied to improve the decay rates. The decay rate of dye in surfactants depends on the Km of surfactants and their ability to offering an effective hydrogen source. The photodegradation of CAD can be divided into three stages: the initial lag stage. the fast degradation stage and the final retardation stage. The lag stage will vanish and the decay rates of dye can be greatly improved by 2.5-3.6 times after adding an additional hydrogen source (NaBH4) or photosensitizer (acetone) to the surfactant micellar solution. However, the use of an additional hydrogen source or photosensitizer has dosage limitations in such applications. The photoreduction of DR is the main reaction mechanism, in which photodechlorination is observed first with the generation of HCI as the final product, then followed by photodecolorization by breaking the azo bond of the chromophore.

Synthesis of Superheavy Nuclei in 48CA-INDUCED Reactions

NASA Astrophysics Data System (ADS)

Oganessian, Yu. Ts.; Utyonkov, V. K.; Lobanov, Yu. V.; Abdullin, F. Sh.; Polyakov, A. N.; Sagaidak, R. N.; Shirokovsky, I. V.; Tsyganov, Yu. S.; Voinov, A. A.; Gulbekian, G. G.; Bogomolov, S. L.; Gikal, B. N.; Mezentsev, A. N.; Iliev, S.; Subbotin, V. G.; Sukhov, A. M.; Subotic, K.; Zagrebaev, V. I.; Vostokin, G. K.; Itkis, M. G.; Moody, K. J.; Patin, J. B.; Shaughnessy, D. A.; Stoyer, M. A.; Stoyer, N. J.; Wilk, P. A.; Kenneally, J. M.; Landrum, J. H.; Wild, J. F.; Lougheed, R. W.

2008-11-01

Thirty-four new nuclides with Z = 104-116, 118 and N = 161-177 have been synthesized in the complete-fusion reactions of 238U, 237Np, 242,244Pu, 243Am, 245,248Cm, and 249Cf targets with 48Ca beams. The masses of evaporation residues were identified through measurements of the excitation functions of the xn-evaporation channels and from cross bombardments. The decay properties of the new nuclei agree with those of previously known heavy nuclei and with predictions from different theoretical models. A discussion of self-consistent interpretations of all observed decay chains originating from the parent isotopes 282,283112, 282113, 286-289114, 287,288115, 290-293116, and 294118 is presented. Decay energies and lifetimes of the neutron-rich superheavy nuclei as well as their production cross sections indicate a considerable increase in the stability of nuclei with an increasing number of neutrons, which agrees with the predictions of theoretical models concerning the decisive dependence of the structure and radioactive properties of superheavy elements on their proximity to the nuclear shells with N = 184 and Z = 114.

Study of the 249-251Cf + 48Ca reactions: recent results and outlook

NASA Astrophysics Data System (ADS)

Voinov, A. A.; Oganessian, Yu Ts; Abdullin, F. Sh; Brewer, N. T.; Dmitriev, S. N.; Grzywacz, R. K.; Hamilton, J. H.; Itkis, M. G.; Miernik, K.; Polyakov, A. N.; Roberto, J. B.; Rykaczewski, K. P.; Sabelnikov, A. V.; Sagaidak, R. N.; Shirokovsky, I. V.; Shumeiko, M. V.; Stoyer, M. A.; Subbotin, V. G.; Sukhov, A. M.; Tsyganov, Yu S.; Utyonkov, V. K.; Vostokin, G. K.

2018-02-01

Experiment aiming at the synthesis of heavy isotopes of Z=118 (Og) using beam of 48Ca and a target of 249-251Cf was undertaken in October 2015 - April 2016 employing the Dubna Gas-Filled Recoil Separator (FLNR JINR). The target of mixed isotopes of 249-251Cf (50.7% of 249Cf, 12.9% of 250Cf, and 36.4% of 251Cf) was irradiated by 48Ca ions at two beam energies of 252 and 258 MeV with the corresponding accumulated beam doses of 1.6×1019 and 1.1×1019. A single event observed at lower beam energy was assigned to the isotope 294Og, the product of the reaction 249Cf(48Ca, 3n); its decay pattern and the observed radioactive properties of the nuclides in the decay chain reproduce in full those observed for 294Og in our earlier experiments of 2002-2005 and 2012. At higher beam energy we observed no decay chains that could be attributed to the isotopes of Og. The possibility of renewal of this experiment in the future is discussed.

Recoil-α-fission and recoil-α-α-fission events observed in the reaction 48Ca + 243Am

NASA Astrophysics Data System (ADS)

Forsberg, U.; Rudolph, D.; Andersson, L.-L.; Di Nitto, A.; Düllmann, Ch. E.; Fahlander, C.; Gates, J. M.; Golubev, P.; Gregorich, K. E.; Gross, C. J.; Herzberg, R.-D.; Heßberger, F. P.; Khuyagbaatar, J.; Kratz, J. V.; Rykaczewski, K.; Sarmiento, L. G.; Schädel, M.; Yakushev, A.; Åberg, S.; Ackermann, D.; Block, M.; Brand, H.; Carlsson, B. G.; Cox, D.; Derkx, X.; Dobaczewski, J.; Eberhardt, K.; Even, J.; Gerl, J.; Jäger, E.; Kindler, B.; Krier, J.; Kojouharov, I.; Kurz, N.; Lommel, B.; Mistry, A.; Mokry, C.; Nazarewicz, W.; Nitsche, H.; Omtvedt, J. P.; Papadakis, P.; Ragnarsson, I.; Runke, J.; Schaffner, H.; Schausten, B.; Shi, Yue; Thörle-Pospiech, P.; Torres, T.; Traut, T.; Trautmann, N.; Türler, A.; Ward, A.; Ward, D. E.; Wiehl, N.

2016-09-01

Products of the fusion-evaporation reaction 48Ca + 243Am were studied with the TASISpec set-up at the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany. Amongst the detected thirty correlated α-decay chains associated with the production of element Z = 115, two recoil-α-fission and five recoil- α- α-fission events were observed. The latter five chains are similar to four such events reported from experiments performed at the Dubna gas-filled separator, and three such events reported from an experiment at the Berkeley gas-filled separator. The four chains observed at the Dubna gas-filled separator were assigned to start from the 2n-evaporation channel 289115 due to the fact that these recoil- α- α-fission events were observed only at low excitation energies. Contrary to this interpretation, we suggest that some of these recoil- α- α-fission decay chains, as well as some of the recoil- α- α-fission and recoil-α-fission decay chains reported from Berkeley and in this article, start from the 3n-evaporation channel 288115.

A novel and facile decay path of Criegee intermediates by intramolecular insertion reactions via roaming transition states

NASA Astrophysics Data System (ADS)

Nguyen, Trong-Nghia; Putikam, Raghunath; Lin, M. C.

2015-03-01

We have discovered a new and highly competitive product channel in the unimolecular decay process for small Criegee intermediates, CH2OO and anti/syn-CH3C(H)OO, occurring by intramolecular insertion reactions via a roaming-like transition state (TS) based on quantum-chemical calculations. Our results show that in the decomposition of CH2OO and anti-CH3C(H)OO, the predominant paths directly produce cis-HC(O)OH and syn-CH3C(O)OH acids with >110 kcal/mol exothermicities via loose roaming-like insertion TSs involving the terminal O atom and the neighboring C-H bonds. For syn-CH3C(H)OO, the major decomposition channel occurs by abstraction of a H atom from the CH3 group by the terminal O atom producing CH2C(H)O-OH. At 298 K, the intramolecular insertion process in CH2OO was found to be 600 times faster than the commonly assumed ring-closing reaction.

ASCA measurements of the grain-scattered X-ray halos of eclipsing massive X-ray binaries: Vela X-1 and Centaurus X-3

NASA Technical Reports Server (NTRS)

Woo, Jonathan W.; Clark, George W.; Day, Charles S. R.; Nagase, Fumiaki; Takeshima, Toshiaki

1994-01-01

We have measured the decaying dust-scattered X-ray halo of Cen X-3 during its binary eclipse with the ASCA solid-state imaging spectrometer (SIS). The surface brightness profile (SBP) of the image in the low-energy band (0.5-3 keV) lies substantially above the point-spread function (PSF) of the X-ray telescope, while the SBP in the high-energy band (5-10 keV) exhibits no significant deviation. By contrast, the SBPs of Vela X-1 during its eclipse are consistent with the PSF in both the low- and high-energy bands -- strong evidence that a dust halo is indeed present in Cen X-3. Accordingly, we modeled the SBP of Cen X-3 taken from six consecutive time segments under the principal assumptions that the dust is distributed uniformly along a segment of the line of sight, the grains have a power-law size distribution, and the low-energy source flux was the same function of orbital phase before as during our observation. The best-fit set of parameters included a grain density value of 1.3 g/cu cm, substanially less than the density of 'astronomical silicate.' This result supports the idea that interstellar grains are 'fluffy' aggregates of smaller solid particles. We attribute the failure to detect a halo of Vela X-1 during its eclipse phase to extended strong circumsource absorption that probably occurred before the eclipse and allowed the halo to decay away before the observation began.

Percolation of binary disk systems: Modeling and theory

DOE PAGES

Meeks, Kelsey; Tencer, John; Pantoya, Michelle L.

2017-01-12

The dispersion and connectivity of particles with a high degree of polydispersity is relevant to problems involving composite material properties and reaction decomposition prediction and has been the subject of much study in the literature. This paper utilizes Monte Carlo models to predict percolation thresholds for a two-dimensional systems containing disks of two different radii. Monte Carlo simulations and spanning probability are used to extend prior models into regions of higher polydispersity than those previously considered. A correlation to predict the percolation threshold for binary disk systems is proposed based on the extended dataset presented in this work and comparedmore » to previously published correlations. Finally, a set of boundary conditions necessary for a good fit is presented, and a condition for maximizing percolation threshold for binary disk systems is suggested.« less

Interactions between multiple supermassive black holes in galactic nuclei: a solution to the final parsec problem

NASA Astrophysics Data System (ADS)

Ryu, Taeho; Perna, Rosalba; Haiman, Zoltán; Ostriker, Jeremiah P.; Stone, Nicholas C.

2018-01-01

Using few-body simulations, we investigate the evolution of supermassive black holes (SMBHs) in galaxies (M* = 1010-1012 M⊙ at z = 0) at 0 < z < 4. Following galaxy merger trees from the Millennium simulation, we model BH mergers with two extreme binary decay scenarios for the 'hard binary' stage: a full or an empty loss cone. These two models should bracket the true evolution, and allow us to separately explore the role of dynamical friction and that of multibody BH interactions on BH mergers. Using the computed merger rates, we infer the stochastic gravitational wave background (GWB). Our dynamical approach is a first attempt to study the dynamical evolution of multiple SMBHs in the host galaxies undergoing mergers with various mass ratios (10-4 < q* < 1). Our main result demonstrates that SMBH binaries are able to merge in both scenarios. In the empty loss cone case, we find that BHs merge via multibody interactions, avoiding the 'final parsec' problem, and entering the pulsar timing arrays band with substantial orbital eccentricity. Our full loss cone treatment, albeit more approximate, suggests that the eccentricity becomes even higher when GWs become dominant, leading to rapid coalescences (binary lifetime ≲1 Gyr). Despite the lower merger rates in the empty loss cone case, due to their higher mass ratios and lower redshifts, the GWB in the full/empty loss cone models are comparable (0.70 × 10-15 and 0.53 × 10-15 at a frequency of 1 yr-1, respectively). Finally, we compute the effects of high eccentricities on the GWB spectrum.

INTRODUCING CAFein, A NEW COMPUTATIONAL TOOL FOR STELLAR PULSATIONS AND DYNAMIC TIDES

DOE Office of Scientific and Technical Information (OSTI.GOV)

Valsecchi, F.; Farr, W. M.; Willems, B.

2013-08-10

Here we present CAFein, a new computational tool for investigating radiative dissipation of dynamic tides in close binaries and of non-adiabatic, non-radial stellar oscillations in isolated stars in the linear regime. For the latter, CAFein computes the non-adiabatic eigenfrequencies and eigenfunctions of detailed stellar models. The code is based on the so-called Riccati method, a numerical algorithm that has been successfully applied to a variety of stellar pulsators, and which does not suffer from the major drawbacks of commonly used shooting and relaxation schemes. Here we present an extension of the Riccati method to investigate dynamic tides in close binaries.more » We demonstrate CAFein's capabilities as a stellar pulsation code both in the adiabatic and non-adiabatic regimes, by reproducing previously published eigenfrequencies of a polytrope, and by successfully identifying the unstable modes of a stellar model in the {beta} Cephei/SPB region of the Hertzsprung-Russell diagram. Finally, we verify CAFein's behavior in the dynamic tides regime by investigating the effects of dynamic tides on the eigenfunctions and orbital and spin evolution of massive main sequence stars in eccentric binaries, and of hot Jupiter host stars. The plethora of asteroseismic data provided by NASA's Kepler satellite, some of which include the direct detection of tidally excited stellar oscillations, make CAFein quite timely. Furthermore, the increasing number of observed short-period detached double white dwarfs (WDs) and the observed orbital decay in the tightest of such binaries open up a new possibility of investigating WD interiors through the effects of tides on their orbital evolution.« less

Measurement of Neutral-Current K + Production by Neutrinos using MINERvA

DOE Office of Scientific and Technical Information (OSTI.GOV)

Marshall, C. M.; Aliaga, L.; Altinok, O.

Neutral-current production of K + by atmospheric neutrinos is a background in searches for the proton decay p → K +ν¯. Reactions such as νp → νK +Λ are indistinguishable from proton decays when the decay products of the Λ are below detection threshold. Events with K + are identified in MINERvA by reconstructing the timing signature of a K + decay at rest. A sample of 201 neutrino-induced neutral-current K + events is used to measure differential cross sections with respect to the K + kinetic energy, and the non-K + hadronic visible energy. An excess of events atmore » low hadronic visible energy is observed relative to the prediction of the neut event generator. Good agreement is observed with the cross section prediction of the genie generator. In conclusion, a search for photons from π 0 decay, which would veto a neutral-current K + event in a proton decay search, is performed, and a 2σ deficit of detached photons is observed relative to the genie prediction.« less

Measurement of Neutral-Current K + Production by Neutrinos using MINERvA

DOE PAGES

Marshall, C. M.; Aliaga, L.; Altinok, O.; ...

2017-07-07

Neutral-current production of K + by atmospheric neutrinos is a background in searches for the proton decay p → K +ν¯. Reactions such as νp → νK +Λ are indistinguishable from proton decays when the decay products of the Λ are below detection threshold. Events with K + are identified in MINERvA by reconstructing the timing signature of a K + decay at rest. A sample of 201 neutrino-induced neutral-current K + events is used to measure differential cross sections with respect to the K + kinetic energy, and the non-K + hadronic visible energy. An excess of events atmore » low hadronic visible energy is observed relative to the prediction of the neut event generator. Good agreement is observed with the cross section prediction of the genie generator. In conclusion, a search for photons from π 0 decay, which would veto a neutral-current K + event in a proton decay search, is performed, and a 2σ deficit of detached photons is observed relative to the genie prediction.« less

Coincidence studies of diffraction structures in binary encounter electron spectra

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liao, C.; Hagmann, S.; Richard, P.

The authors have measured binary encounter electron (BEe) production in collisions of 0.3 MeV/u Cu{sup q+} (q=4,12) projectiles on H{sub 2} targets from 0 to 70 degrees with respect to the beam direction. Prominent features are the appearance of the BEe peak splitting and a very strong forward peaked angular distribution which are attributed to the diffractive scattering of the quasifree target electrons in the short range potential of the projectile. Using electron-projectile final charge state coincidence techniques, different collision reaction channels can be separated. Measurements of this type are being pursued.

The reactions of cytidine and 2'-deoxycytidine with SO4.- revisited. Pulse radiolysis and product studies.

PubMed

Aravindakumar, Charuvila T; Schuchmann, Man Nien; Rao, Balijepalli S; von Sonntag, Justus; von Sonntag, Clemens

2003-01-21

The reactions of SO4.- with 2'-deoxycytidine 1a and cytidine 1b lead to very different intermediates (base radicals with 1a, sugar radicals with 1b). The present study provides spectral and kinetic data for the various intermediates by pulse radiolysis as well as information on final product yields (free cytosine). Taking these and literature data into account allows us to substantiate but also modify in essential aspects the current mechanistic concept (H. Catterall, M. J. Davies and B. C. Gilbert, J. Chem. Soc., Perkin Trans. 2, 1992, 1379). SO4.- radicals have been generated radiolytically in the reaction of peroxodisulfate with the hydrated electron (and the H. atom). In the reaction of SO4.- with 1a (k = 1.6 x 10(9) dm3 mol-1 s-1), a transient (lambda max = 400 nm, shifted to 450 nm at pH 3) is observed. This absorption is due to two intermediates. The major component (lambda max approximately 385 nm) does not react with O2 and has been attributed to an N-centered radical 4a formed upon sulfate release and deprotonation at nitrogen. The minor component, rapidly wiped out by O2, must be due to C-centered OH-adduct radical(s) 6a and/or 7a suggested to be formed by a water-induced nucleophilic replacement. These radicals decay by second-order kinetics. Free cytosine is only formed in low yields (G = 0.14 x 10(-7) mol J-1 upon electron-beam irradiation). In contrast, 1b gives rise to an intermediate absorbing at lambda max = 530 nm (shifted to 600 nm in acid solution) which rapidly decays (k = 6 x 10(4) s-1). In the presence of O2, the decay is much faster (k approximately 1.3 x 10(9) dm3 mol-1 s-1) indicating that this species must be a C-centered radical. This has been attributed to the C(5)-yl radical 8 formed upon the reaction of the C(2')-OH group with the cytidine SO4(.-)-adduct radical 2b. This reaction competes very effectively with the corresponding reaction of water and the release of sulfate and a proton generating the N-centered radical. Upon the decay of 8, sugar radical 11 is formed with the release of cytosine. The latter is formed with a G value of 2.8 x 10(-7) mol J-1 (85% of primary SO4.-) at high dose rates (electron beam irradiation). At low dose rates (gamma-radiolysis) its yield is increased to 7 x 10(-7) mol J-1 due to a chain reaction involving peroxodisulfate and reducing free radicals. Phosphate buffer prevents the formation of the sugar radical at the SO4(.-)-adduct stage by enhancing the rate of sulfate release by deprotonation of 2b and also by speeding up the decay of the C(5)-yl radical into another (base) radical. Cytosine release in cytidine is mechanistically related to strand breakage in poly(C). Literature data on the effect of dioxygen on strand breakage yields in poly(C) induced by SO4.- (suppressed) and upon photoionisation (unaltered) lead us to conclude that in poly(C) and also in the present system free radical cations are not involved to a major extent. This conclusion modifies an essential aspect of the current mechanistic concept.

Critical fluid light scattering

NASA Technical Reports Server (NTRS)

Gammon, Robert W.

1988-01-01

The objective is to measure the decay rates of critical density fluctuations in a simple fluid (xenon) very near its liquid-vapor critical point using laser light scattering and photon correlation spectroscopy. Such experiments were severely limited on Earth by the presence of gravity which causes large density gradients in the sample when the compressibility diverges approaching the critical point. The goal is to measure fluctuation decay rates at least two decades closer to the critical point than is possible on earth, with a resolution of 3 microK. This will require loading the sample to 0.1 percent of the critical density and taking data as close as 100 microK to the critical temperature. The minimum mission time of 100 hours will allow a complete range of temperature points to be covered, limited by the thermal response of the sample. Other technical problems have to be addressed such as multiple scattering and the effect of wetting layers. The experiment entails measurement of the scattering intensity fluctuation decay rate at two angles for each temperature and simultaneously recording the scattering intensities and sample turbidity (from the transmission). The analyzed intensity and turbidity data gives the correlation length at each temperature and locates the critical temperature. The fluctuation decay rate data from these measurements will provide a severe test of the generalized hydrodynamic theories of transport coefficients in the critical regions. When compared to equivalent data from binary liquid critical mixtures they will test the universality of critical dynamics.

Nuclear Data Sheets for A = 148

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nica, N.

2014-04-02

The experimental nuclear structure data available through October 2013 have been reviewed. A summary of information obtained in various reaction and decay experiments is presented, together with adopted level schemes.

Trojan horse particle invariance: The impact on nuclear astrophysics

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pizzone, R. G.; La Cognata, M.; Spitaleri, C.

In the current picture of nuclear astrophysics indirect methods and, in particular, the Trojan Horse Method cover a crucial role for the measurement of charged particle induced reactions cross sections of astrophysical interest, in the energy range required by the astrophysical scenarios. To better understand its cornerstones and its applications to physical cases many tests were performed to verify all its properties and the possible future perspectives. The key to the method is the quasi-free break-up and some of its properties will be investigated in the present work. In particular, the Trojan Horse nucleus invariance will be studied and previousmore » studies will be extended to the cases of the binary d(d, p)t and {sup 6}Li(d,α){sup 4}He reactions, which were tested using different quasi-free break-up's, namely {sup 6}Li and {sup 3}He. The astrophysical S(E)-factor were then extracted with the Trojan Horse formalism applied to the two different break-up schemes and compared with direct data as well as with previous indirect investigations. The very good agreement confirms the independence of binary indirect cross section on the chosen spectator particle also for these reactions.« less

Buoyancy effects on the radiative magneto Micropolar nanofluid flow with double stratification, activation energy and binary chemical reaction.

PubMed

Ramzan, M; Ullah, Naeem; Chung, Jae Dong; Lu, Dianchen; Farooq, Umer

2017-10-10

A mathematical model has been developed to examine the magneto hydrodynamic micropolar nanofluid flow with buoyancy effects. Flow analysis is carried out in the presence of nonlinear thermal radiation and dual stratification. The impact of binary chemical reaction with Arrhenius activation energy is also considered. Apposite transformations are engaged to transform nonlinear partial differential equations to differential equations with high nonlinearity. Resulting nonlinear system of differential equations is solved by differential solver method in Maple software which uses Runge-Kutta fourth and fifth order technique (RK45). To authenticate the obtained results, a comparison with the preceding article is also made. The evaluations are executed graphically for numerous prominent parameters versus velocity, micro rotation component, temperature, and concentration distributions. Tabulated numerical calculations of Nusselt and Sherwood numbers with respective well-argued discussions are also presented. Our findings illustrate that the angular velocity component declines for opposing buoyancy forces and enhances for aiding buoyancy forces by changing the micropolar parameter. It is also found that concentration profile increases for higher values of chemical reaction parameter, whereas it diminishes for growing values of solutal stratification parameter.

New Fragment Separation Technology for Superheavy Element Research

DOE Office of Scientific and Technical Information (OSTI.GOV)

Shaughnessy, D A; Moody, K J; Henderson, R A

2008-01-28

This project consisted of three major research areas: (1) development of a solid Pu ceramic target for the MASHA separator, (2) chemical separation of nuclear decay products, and (3) production of new isotopes and elements through nuclear reactions. There have been 16 publications as a result of this project, and this collection of papers summarizes our accomplishments in each of the three areas of research listed above. The MASHA (Mass Analyzer for Super-Heavy Atoms) separator is being constructed at the U400 Cyclotron at the Flerov Laboratory of Nuclear Reactions in Dubna, Russia. The purpose of the separator is to physicallymore » separate the products from nuclear reactions based on their isotopic masses rather than their decay characteristics. The separator was designed to have a separation between isotopic masses of {+-}0.25 amu, which would enable the mass of element 114 isotopes to be measured with outstanding resolution, thereby confirming their discovery. In order to increase the production rate of element 114 nuclides produced via the {sup 244}Pu+{sup 48}Ca reaction, a new target technology was required. Instead of a traditional thin actinide target, the MASHA separator required a thick, ceramic-based Pu target that was thick enough to increase element 114 production while still being porous enough to allow reaction products to migrate out of the target and travel through the separator to the detector array located at the back end. In collaboration with UNLV, we began work on development of the Pu target for MASHA. Using waste-form synthesis technology, we began by creating zirconia-based matrices that would form a ceramic with plutonium oxide. We used samarium oxide as a surrogate for Pu and created ceramics that had varying amounts of the starting materials in order to establish trends in material density and porosity. The results from this work are described in more detail in Refs. [1,4,10]. Unfortunately, work on MASHA was delayed in Russia because it was found that the efficiency of transporting products from the target chamber to the detector array was much too low for applications in heavy element experiments where production rates are on the order of one atom per day or less. Work continues on the MASHA separator, and once the efficiency has been improved, we plan to continue our work on the Pu target for future element 114 experiments. Due to the delays of the MASHA separator, work on establishing the identity of heavy element species produced through nuclear reactions focused instead on chemical separations. In particular, element 115 decays through a series of alpha decays, terminating with an element 105 isotope with a long half-life ({approx} 1 day). By chemically separating the element 105 daughter and observing its subsequent fission decay, the identity of the original parent nucleus can be established through the genetic correlation of the initial series of alpha decays. Chemical separations of element 105 were developed in Switzerland, Russia, and at LLNL. Over the course of two experiments, reaction products from the {sup 243}Am+{sup 48}Ca reaction were collected in a copper block and subsequently processed for chemical separation of the Group Five elements [8,9,13,15]. The Group Five elements were initially separated from the Group Four species, and then the samples were sub-divided into tantalum and niobium fractions. All of the fission events were observed in the tantalum fractions, which implied that element 105 behaved more like tantalum under the chemical conditions of these experiments. These experiments were very successful, and not only demonstrated that chemical separation could be performed on single atoms of interest, but also lent proof to the identity of the parent nucleus as element 115. Subsequent analysis of the alpha spectra taken during the experiment further prove that the fission events observed during the two experiments came from element 105 as the decay daughter of element 115 and could not attributed to interference from other background species [16]. The final aspect of this project was the production of new isotopes and elements. All of the experiments were performed in Dubna at the U400 Cyclotron and the results are described in more detail in Refs. [2,3,5-8,11,12,14]. The first experiments were designed to establish the decay properties of isotopes of elements 112, 114, and 116 [5]. Because these isotopic signatures were established through these initial experiments, the discovery of element 118 [11] was possible, since the 118 nuclides decayed into these previously studied isotopes. This was the first successful report of the discovery of element 118, which was reported by the media to a large extent. The last experiment that was performed for this project was the production and detection of a new isotope of element 113 [14].« less

Test of the Brink-Axel Hypothesis for the Pygmy Dipole Resonance

NASA Astrophysics Data System (ADS)

Martin, D.; von Neumann-Cosel, P.; Tamii, A.; Aoi, N.; Bassauer, S.; Bertulani, C. A.; Carter, J.; Donaldson, L.; Fujita, H.; Fujita, Y.; Hashimoto, T.; Hatanaka, K.; Ito, T.; Krugmann, A.; Liu, B.; Maeda, Y.; Miki, K.; Neveling, R.; Pietralla, N.; Poltoratska, I.; Ponomarev, V. Yu.; Richter, A.; Shima, T.; Yamamoto, T.; Zweidinger, M.

2017-11-01

The gamma strength function and level density of 1- states in 96Mo have been extracted from a high-resolution study of the (p → , p→ ' ) reaction at 295 MeV and extreme forward angles. By comparison with compound nucleus γ decay experiments, this allows a test of the generalized Brink-Axel hypothesis in the energy region of the pygmy dipole resonance. The Brink-Axel hypothesis is commonly assumed in astrophysical reaction network calculations and states that the gamma strength function in nuclei is independent of the structure of the initial and final state. The present results validate the Brink-Axel hypothesis for 96Mo and provide independent confirmation of the methods used to separate gamma strength function and level density in γ decay experiments.

Synthesis of superheavy elements at the Dubna gas-filled recoil separator

NASA Astrophysics Data System (ADS)

Voinov, A. A.

2016-12-01

A survey of experiments at the Dubna gas-filled recoil separator (Laboratory of Nuclear Reactions, JINR, Dubna) aimed at the detection and study of the "island of stability" of superheavy nuclei produced in complete fusion reactions of 48Ca ions and 238U-249Cf target nuclei is given. The problems of synthesis of superheavy nuclei, methods for their identification, and investigation of their decay properties, including the results of recent experiments at other separators (SHIP, BGS, TASCA) and chemical setups, are discussed. The studied properties of the new nuclei, the isotopes of elements 112-118, as well as the properties of their decay products, indicate substantial growth of stability of the heaviest nuclei with increasing number of neutrons in the nucleus as the magic number of neutrons N = 184 is approached.

Heavy-quark production and elliptic flow in Au+Au collisions at √s NN=62.4 GeV

DOE PAGES

Adare, A.

2015-04-28

In this study, we present measurements of electrons and positrons from the semileptonic decays of heavy-flavor hadrons at midrapidity (|y|< 0.35) in Au+Au collisions at √s NN = 62.4 GeV. The data were collected in 2010 by the PHENIX experiment that included the new hadron-blind detector. The invariant yield of electrons from heavy-flavor decays is measured as a function of transverse momentum in the range 1 < p e T < 5 GeV/c. The invariant yield per binary collision is slightly enhanced above the p+p reference in Au+Au 0%–20%, 20%–40%, and 40%–60% centralities at a comparable level. At this lowmore » beam energy this may be a result of the interplay between initial-state Cronin effects, final-state flow, and energy loss in medium. The v₂ of electrons from heavy-flavor decays is nonzero when averaged between 1.3 < p e T < 2.5 GeV/c for 0%–40% centrality collisions at √s NN = 62.4 GeV. For 20%–40% centrality collisions, the v₂ at √s NN = 62.4 GeV is smaller than that for heavy-flavor decays at √s NN = 200 GeV. The v₂ of the electrons from heavy-flavor decay at the lower beam energy is also smaller than v₂ for pions. Both results indicate that the heavy-quarks interact with the medium formed in these collisions, but they may not be at the same level of thermalization with the medium as observed at √s NN = 200 GeV.« less

Heavy-quark production and elliptic flow in Au + Au collisions at √{sN N}=62.4 GeV

NASA Astrophysics Data System (ADS)

Adare, A.; Aidala, C.; Ajitanand, N. N.; Akiba, Y.; Akimoto, R.; Al-Ta'Ani, H.; Alexander, J.; Angerami, A.; Aoki, K.; Apadula, N.; Aramaki, Y.; Asano, H.; Aschenauer, E. C.; Atomssa, E. T.; Awes, T. C.; Azmoun, B.; Babintsev, V.; Bai, M.; Bannier, B.; Barish, K. N.; Bassalleck, B.; Bathe, S.; Baublis, V.; Baumgart, S.; Bazilevsky, A.; Belmont, R.; Berdnikov, A.; Berdnikov, Y.; Bing, X.; Blau, D. S.; Bok, J. S.; Boyle, K.; Brooks, M. L.; Buesching, H.; Bumazhnov, V.; Butsyk, S.; Campbell, S.; Castera, P.; Chen, C.-H.; Chi, C. Y.; Chiu, M.; Choi, I. J.; Choi, J. B.; Choi, S.; Choudhury, R. K.; Christiansen, P.; Chujo, T.; Chvala, O.; Cianciolo, V.; Citron, Z.; Cole, B. A.; Connors, M.; Csanád, M.; Csörgő, T.; Dairaku, S.; Datta, A.; Daugherity, M. S.; David, G.; Denisov, A.; Deshpande, A.; Desmond, E. J.; Dharmawardane, K. V.; Dietzsch, O.; Ding, L.; Dion, A.; Donadelli, M.; Drapier, O.; Drees, A.; Drees, K. A.; Durham, J. M.; Durum, A.; D'Orazio, L.; Edwards, S.; Efremenko, Y. V.; Engelmore, T.; Enokizono, A.; Esumi, S.; Eyser, K. O.; Fadem, B.; Fields, D. E.; Finger, M.; Finger, M.; Fleuret, F.; Fokin, S. L.; Frantz, J. E.; Franz, A.; Frawley, A. D.; Fukao, Y.; Fusayasu, T.; Gainey, K.; Gal, C.; Garishvili, A.; Garishvili, I.; Glenn, A.; Gong, X.; Gonin, M.; Goto, Y.; Granier de Cassagnac, R.; Grau, N.; Greene, S. V.; Grosse Perdekamp, M.; Gunji, T.; Guo, L.; Gustafsson, H.-Å.; Hachiya, T.; Haggerty, J. S.; Hahn, K. I.; Hamagaki, H.; Hanks, J.; Hashimoto, K.; Haslum, E.; Hayano, R.; He, X.; Hemmick, T. K.; Hester, T.; Hill, J. C.; Hollis, R. S.; Homma, K.; Hong, B.; Horaguchi, T.; Hori, Y.; Huang, S.; Ichihara, T.; Iinuma, H.; Ikeda, Y.; Imrek, J.; Inaba, M.; Iordanova, A.; Isenhower, D.; Issah, M.; Ivanishchev, D.; Jacak, B. V.; Javani, M.; Jia, J.; Jiang, X.; Johnson, B. M.; Joo, K. S.; Jouan, D.; Jumper, D. S.; Kamin, J.; Kaneti, S.; Kang, B. H.; Kang, J. H.; Kang, J. S.; Kapustinsky, J.; Karatsu, K.; Kasai, M.; Kawall, D.; Kazantsev, A. V.; Kempel, T.; Khanzadeev, A.; Kijima, K. M.; Kim, B. I.; Kim, C.; Kim, D. J.; Kim, E.-J.; Kim, H. J.; Kim, K.-B.; Kim, Y.-J.; Kim, Y. K.; Kinney, E.; Kiss, Á.; Kistenev, E.; Klatsky, J.; Kleinjan, D.; Kline, P.; Komatsu, Y.; Komkov, B.; Koster, J.; Kotchetkov, D.; Kotov, D.; Král, A.; Krizek, F.; Kunde, G. J.; Kurita, K.; Kurosawa, M.; Kwon, Y.; Kyle, G. S.; Lacey, R.; Lai, Y. S.; Lajoie, J. G.; Lebedev, A.; Lee, B.; Lee, D. M.; Lee, J.; Lee, K. B.; Lee, K. S.; Lee, S. H.; Lee, S. R.; Leitch, M. J.; Leite, M. A. L.; Leitgab, M.; Lewis, B.; Lim, S. H.; Linden Levy, L. A.; Liu, M. X.; Love, B.; Maguire, C. F.; Makdisi, Y. I.; Makek, M.; Manion, A.; Manko, V. I.; Mannel, E.; Masumoto, S.; McCumber, M.; McGaughey, P. L.; McGlinchey, D.; McKinney, C.; Mendoza, M.; Meredith, B.; Miake, Y.; Mibe, T.; Mignerey, A. C.; Milov, A.; Mishra, D. K.; Mitchell, J. T.; Miyachi, Y.; Miyasaka, S.; Mohanty, A. K.; Moon, H. J.; Morrison, D. P.; Motschwiller, S.; Moukhanova, T. V.; Murakami, T.; Murata, J.; Nagae, T.; Nagamiya, S.; Nagle, J. L.; Nagy, M. I.; Nakagawa, I.; Nakamiya, Y.; Nakamura, K. R.; Nakamura, T.; Nakano, K.; Nattrass, C.; Nederlof, A.; Nihashi, M.; Nouicer, R.; Novitzky, N.; Nyanin, A. S.; O'Brien, E.; Ogilvie, C. A.; Okada, K.; Oskarsson, A.; Ouchida, M.; Ozawa, K.; Pak, R.; Pantuev, V.; Papavassiliou, V.; Park, B. H.; Park, I. H.; Park, S. K.; Pate, S. F.; Patel, L.; Pei, H.; Peng, J.-C.; Pereira, H.; Peressounko, D. Yu.; Petti, R.; Pinkenburg, C.; Pisani, R. P.; Proissl, M.; Purschke, M. L.; Qu, H.; Rak, J.; Ravinovich, I.; Read, K. F.; Reynolds, D.; Riabov, V.; Riabov, Y.; Richardson, E.; Riveli, N.; Roach, D.; Roche, G.; Rolnick, S. D.; Rosati, M.; Sahlmueller, B.; Saito, N.; Sakaguchi, T.; Samsonov, V.; Sano, M.; Sarsour, M.; Sawada, S.; Sedgwick, K.; Seidl, R.; Sen, A.; Seto, R.; Sharma, D.; Shein, I.; Shibata, T.-A.; Shigaki, K.; Shimomura, M.; Shoji, K.; Shukla, P.; Sickles, A.; Silva, C. L.; Silvermyr, D.; Sim, K. S.; Singh, B. K.; Singh, C. P.; Singh, V.; Slunečka, M.; Soltz, R. A.; Sondheim, W. E.; Sorensen, S. P.; Soumya, M.; Sourikova, I. V.; Stankus, P. W.; Stenlund, E.; Stepanov, M.; Ster, A.; Stoll, S. P.; Sugitate, T.; Sukhanov, A.; Sun, J.; Sziklai, J.; Takagui, E. M.; Takahara, A.; Taketani, A.; Tanaka, Y.; Taneja, S.; Tanida, K.; Tannenbaum, M. J.; Tarafdar, S.; Taranenko, A.; Tennant, E.; Themann, H.; Todoroki, T.; Tomášek, L.; Tomášek, M.; Torii, H.; Towell, R. S.; Tserruya, I.; Tsuchimoto, Y.; Tsuji, T.; Vale, C.; van Hecke, H. W.; Vargyas, M.; Vazquez-Zambrano, E.; Veicht, A.; Velkovska, J.; Vértesi, R.; Virius, M.; Vossen, A.; Vrba, V.; Vznuzdaev, E.; Wang, X. R.; Watanabe, D.; Watanabe, K.; Watanabe, Y.; Watanabe, Y. S.; Wei, F.; Wei, R.; Whitaker, S.; White, S. N.; Winter, D.; Wolin, S.; Woody, C. L.; Wysocki, M.; Yamaguchi, Y. L.; Yang, R.; Yanovich, A.; Ying, J.; Yokkaichi, S.; You, Z.; Younus, I.; Yushmanov, I. E.; Zajc, W. A.; Zelenski, A.; Phenix Collaboration

2015-04-01

We present measurements of electrons and positrons from the semileptonic decays of heavy-flavor hadrons at midrapidity (|y |< 0.35) in Au +Au collisions at √{sN N}=62.4 GeV. The data were collected in 2010 by the PHENIX experiment that included the new hadron-blind detector. The invariant yield of electrons from heavy-flavor decays is measured as a function of transverse momentum in the range 1

Fusion-fission and quasifission in the reactions with heavy ions leading to the formation of Hs

NASA Astrophysics Data System (ADS)

Itkis, I. M.; Itkis, M. G.; Knyazheva, G. N.; Kozulin, E. M.

2012-10-01

Mass and energy distributions of binary reaction products obtained in the reactions 22Ne+249Cf,26Mg+248Cm,36S+238U and 58Fe+208Pb leading to Hs isotopes have been measured. At energies below the Coulomb barrier the bimodal fission of Hs*, formed in the reaction 26Mg+248Cm, is observed. In the reaction 36S+238U the considerable part of the symmetric fragments arises from the quasifission process. At energies above the Coulomb barrier the symmetric fragments originate mainly from fusion-fission process for both reactions with Mg and S ions. In the case of the 58Fe+208Pb reaction the quasifission process dominates at all measured energies. The pre- and post-scission neutron multiplicities as a function of the fragment mass have been obtained for the reactions studied.

Beta-delayed proton emission from 20Mg

NASA Astrophysics Data System (ADS)

Lund, M. V.; Andreyev, A.; Borge, M. J. G.; Cederkäll, J.; De Witte, H.; Fraile, L. M.; Fynbo, H. O. U.; Greenlees, P. T.; Harkness-Brennan, L. J.; Howard, A. M.; Huyse, M.; Jonson, B.; Judson, D. S.; Kirsebom, O. S.; Konki, J.; Kurcewicz, J.; Lazarus, I.; Lica, R.; Lindberg, S.; Madurga, M.; Marginean, N.; Marginean, R.; Marroquin, I.; Mihai, C.; Munch, M.; Nacher, E.; Negret, A.; Nilsson, T.; Page, R. D.; Pascu, S.; Perea, A.; Pucknell, V.; Rahkila, P.; Rapisarda, E.; Riisager, K.; Rotaru, F.; Sotty, C.; Stanoiu, M.; Tengblad, O.; Turturica, A.; Van Duppen, P.; Vedia, V.; Wadsworth, R.; Warr, N.

2016-10-01

Beta-delayed proton emission from 20 Mg has been measured at ISOLDE, CERN, with the ISOLDE Decay Station (IDS) setup including both charged-particle and gamma-ray detection capabilities. A total of 27 delayed proton branches were measured including seven so far unobserved. An updated decay scheme, including three new resonances above the proton separation energy in 20 Na and more precise resonance energies, is presented. Beta-decay feeding to two resonances above the Isobaric Analogue State (IAS) in 20 Na is observed. This may allow studies of the 4032.9(2.4)keV resonance in 19 Ne through the beta decay of 20 Mg, which is important for the astrophysically relevant reaction 15O( α, γ)19Ne . Beta-delayed protons were used to obtain a more precise value for the half-life of 20 Mg, 91.4(1.0)ms.

Study of nitrogen flowing afterglow with mercury vapor injection

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mazánková, V., E-mail: mazankova@fch.vutbr.cz; Krčma, F.; Trunec, D.

2014-10-21

The reaction kinetics in nitrogen flowing afterglow with mercury vapor addition was studied by optical emission spectroscopy. The DC flowing post-discharge in pure nitrogen was created in a quartz tube at the total gas pressure of 1000 Pa and discharge power of 130 W. The mercury vapors were added into the afterglow at the distance of 30 cm behind the active discharge. The optical emission spectra were measured along the flow tube. Three nitrogen spectral systems – the first positive, the second positive, and the first negative, and after the mercury vapor addition also the mercury resonance line at 254more » nm in the spectrum of the second order were identified. The measurement of the spatial dependence of mercury line intensity showed very slow decay of its intensity and the decay rate did not depend on the mercury concentration. In order to explain this behavior, a kinetic model for the reaction in afterglow was developed. This model showed that the state Hg(6 {sup 3}P{sub 1}), which is the upper state of mercury UV resonance line at 254 nm, is produced by the excitation transfer from nitrogen N{sub 2}(A{sup 3}Σ{sup +}{sub u}) metastables to mercury atoms. However, the N{sub 2}(A{sup 3}Σ{sup +}{sub u}) metastables are also produced by the reactions following the N atom recombination, and this limits the decay of N{sub 2}(A{sup 3}Σ{sup +}{sub u}) metastable concentration and results in very slow decay of mercury resonance line intensity. It was found that N atoms are the most important particles in this late nitrogen afterglow, their volume recombination starts a chain of reactions which produce excited states of molecular nitrogen. In order to explain the decrease of N atom concentration, it was also necessary to include the surface recombination of N atoms to the model. The surface recombination was considered as a first order reaction and wall recombination probability γ = (1.35 ± 0.04) × 10{sup −6} was determined from the experimental data. Also sensitivity analysis was applied for the analysis of kinetic model in order to reveal the main control parameters in the model.« less

Effect of the physicochemical properties of binary ionic liquids on lipase activity and stability.

PubMed

Yao, Peipei; Yu, Xinxin; Huang, Xirong

2015-01-01

In the present study, the lipase-catalyzed hydrolysis of p-nitrophenyl butyrate is used as a model reaction to determine the activity and stability of Candida rugosa lipase in binary ionic liquids (ILs). The binary ILs consist of hydrophobic 1-butyl-3-methylimidazolium hexafluorophosphate ([Bmim]PF6) and a small amount of hydrophilic 1-butyl-3-methylimidazolium nitrate ([Bmim]NO3) or 1-butyl-3-methylimidazolium trifluoromethanesulfonate ([Bmim]CF3SO3) or 1-butyl-3-methylimidazolium tetrafluoroborate ([Bmim]BF4). The activity and the stability of lipase are first correlated with the physicochemical properties of the binary ILs. In the three binary IL systems, both the hydrophilicity and the polarity of the systems increase with the increase of the content of hydrophilic ILs (HILs). At a fixed concentration of HIL, they vary in a descending order of [Bmim]PF6/[Bmim]NO3>[Bmim]PF6/[Bmim]CF3SO3>[Bmim]PF6/[Bmim]BF4. This order is in contrast with the order of the lipase conformation stability, i.e., the higher the polarity of ILs, the more unstable the lipase conformation. However, both the activity and the stability of lipase depend on the type and the content of the HIL in binary ILs, showing a complex dependency. Analysis shows that the catalytic performance of lipase in the binary ILs is affected not only by the direct influence of the ILs on lipase conformation, but also through their indirect influence on the physicochemical properties of water. The present study helps to explore binary IL mixtures suitable for lipase-based biocatalysis. Copyright © 2015 Elsevier B.V. All rights reserved.

On the resonant detonation of sub-Chandrasekhar mass white dwarfs during binary inspiral

NASA Astrophysics Data System (ADS)

McKernan, B.; Ford, K. E. S.

2016-12-01

White dwarfs (WDs) are believed to detonate via explosive Carbon-fusion in a Type Ia supernova (SN) when their temperature and/or density reach the point where Carbon is ignited in a runaway reaction. Observations of the Type Ia SN rate imply that all WD binaries that merge through the emission of gravitational radiation within a Hubble time should result in SNe, regardless of total mass. Here we investigate the conditions under which a single WD in a binary system might extract energy from its orbit, depositing enough energy into a resonant mode such that it detonates before merger. We show that, ignoring non-linear effects in a WD binary in tidal lock at small binary separations, the sustained tidal forcing of a low-order quadrupolar g mode or a harmonic of a low-order quadrupolar p mode could, in principle, drive the average temperature of Carbon nuclei in the mode over the runaway fusion threshold. If growing mode energy is thermalized at a core/atmosphere boundary, rapid Helium burning and inwards-travelling p-waves may result in core detonation. Thermalization at a boundary in the core can also result in detonation. If energy can be efficiently transferred from the orbit to modes as the WD binary passes through resonances, the WD merger time-scale will be shortened by Myr-Gyr compared to expected time-scales from gravitational wave (GW)-emission alone and GW detectors will observe deviations from predicted chirp profiles in resolved WD binaries. Future work in this area should focus on whether tidal locking in WD binaries is naturally driven towards low-order mode frequencies.

Accounting for the Decreasing Reaction Potential of Heterogeneous Aquifers in a Stochastic Framework of Aquifer-Scale Reactive Transport

NASA Astrophysics Data System (ADS)

Loschko, Matthias; Wöhling, Thomas; Rudolph, David L.; Cirpka, Olaf A.

2018-01-01

Many groundwater contaminants react with components of the aquifer matrix, causing a depletion of the aquifer's reactivity with time. We discuss conceptual simplifications of reactive transport that allow the implementation of a decreasing reaction potential in reactive-transport simulations in chemically and hydraulically heterogeneous aquifers without relying on a fully explicit description. We replace spatial coordinates by travel-times and use the concept of relative reactivity, which represents the reaction-partner supply from the matrix relative to a reference. Microorganisms facilitating the reactions are not explicitly modeled. Solute mixing is neglected. Streamlines, obtained by particle tracking, are discretized in travel-time increments with variable content of reaction partners in the matrix. As exemplary reactive system, we consider aerobic respiration and denitrification with simplified reaction equations: Dissolved oxygen undergoes conditional zero-order decay, nitrate follows first-order decay, which is inhibited in the presence of dissolved oxygen. Both reactions deplete the bioavailable organic carbon of the matrix, which in turn determines the relative reactivity. These simplifications reduce the computational effort, facilitating stochastic simulations of reactive transport on the aquifer scale. In a one-dimensional test case with a more detailed description of the reactions, we derive a potential relationship between the bioavailable organic-carbon content and the relative reactivity. In a three-dimensional steady-state test case, we use the simplified model to calculate the decreasing denitrification potential of an artificial aquifer over 200 years in an ensemble of 200 members. We demonstrate that the uncertainty in predicting the nitrate breakthrough in a heterogeneous aquifer decreases with increasing scale of observation.

A new measurement of the rare decay eta -> pi^0 gamma gamma with the Crystal Ball/TAPS detectors at the Mainz Microtron

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nefkens, B M; Prakhov, S; Aguar-Bartolom��, P

2014-08-01

A new measurement of the rare, doubly radiative decay eta->pi^0 gamma gamma was conducted with the Crystal Ball and TAPS multiphoton spectrometers together with the photon tagging facility at the Mainz Microtron MAMI. New data on the dependence of the partial decay width, Gamma(eta->pi^0 gamma gamma), on the two-photon invariant mass squared, m^2(gamma gamma), as well as a new, more precise value for the decay width, Gamma(eta->pi^0 gamma gamma) = (0.33+/-0.03_tot) eV, are based on analysis of 1.2 x 10^3 eta->pi^0 gamma gamma decays from a total of 6 x 10^7 eta mesons produced in the gamma p -> etamore » p reaction. The present results for dGamma(eta->pi^0 gamma gamma)/dm^2(gamma gamma) are in good agreement with previous measurements and recent theoretical calculations for this dependence.« less

Beta Decay Study of the Tz = - 256Zn Nucleus and the Determination of the Half-Lives of a Few fp-shell Nuclei

NASA Astrophysics Data System (ADS)

Rubio, B.; Orrigo, S. E. A.; Kucuk, L.; Montaner-Pizá, A.; Fujita, Y.; Fujita, H.; Blank, B.; Gelletly, W.; Adachi, T.; Agramunt, J.; Algora, A.; Ascher, P.; Bilgier, B.; Cáceres, L.; Cakirli, R. B.; de France, G.; Ganioğlu, E.; Gerbaux, M.; Giovinazzo, J.; Grevy, S.; Kamalou, O.; Kozer, H. C.; Kurtukian-Nieto, T.; Marqués, F. M.; Molina, F.; Oktem, Y.; de Oliveira Santos, F.; Perrot, L.; Popescu, L.; Raabe, R.; Rogers, A. M.; Srivastava, P. C.; Susoy, G.; Suzuki, T.; Tamii, A.; Thomas, J. C.

2014-06-01

This paper concerns the experimental study of the β decay properties of few proton-rich fp-shell nuclei. The nuclei were produced at GANIL in fragmentation reactions, separated with the LISE spectrometer and stopped in an implantation detector surrounded by Ge detectors. The β-delayed gammas, β-delayed protons and the exotic β-delayed gamma-proton emission have been studied. Preliminary results are presented. The decay of the Tz = - 2 nucleus 56Zn has been studied in detail. Information from the β-delayed protons and β-delayed gammas has been used to deduce the decay scheme. The exotic beta-delayed gamma-proton decay has been observed for the first time in the fp-shell. The interpretation of the data was made possible thanks to the detailed knowledge of the mirror Charge Exchange (CE) process and the gamma de-excitation of the states in 56Co, the mirror nucleus of 56Cu.

What Is A Homosexual? A Definitional Model.

ERIC Educational Resources Information Center

Berger, Raymond M.

1983-01-01

Presents a definitional model to explain homosexuality and discusses its implications for practice. Contends that social workers must discard the traditional binary model of hetersexual versus homesexual for one incorporating relevant psychosocial factors including life experiences, social reaction, and association with others. (Author/JAC)

Test and Evaluation Management Guide

DTIC Science & Technology

1993-08-01

between Ser- biotoxicity . Chemical-mixing tests are con- vice and DOE test personnel (Reference ducted to obtain information on the binary 55). chemical...reaction. Biotoxicity tests are per- formed to assess the potency of the agent Since the United States signed and ratified generated. Chemical weapons

First measurement of coherent ϕ -meson photoproduction from 4He near threshold

NASA Astrophysics Data System (ADS)

Hiraiwa, T.; Yosoi, M.; Niiyama, M.; Morino, Y.; Nakatsugawa, Y.; Sumihama, M.; Ahn, D. S.; Ahn, J. K.; Chang, W. C.; Chen, J. Y.; Daté, S.; Fujimura, H.; Fukui, S.; Hicks, K.; Hotta, T.; Hwang, S. H.; Ishikawa, T.; Kato, Y.; Kawai, H.; Kohri, H.; Kon, Y.; Lin, P. J.; Maeda, Y.; Miyabe, M.; Mizutani, K.; Muramatsu, N.; Nakano, T.; Nozawa, Y.; Ohashi, Y.; Ohta, T.; Oka, M.; Rangacharyulu, C.; Ryu, S. Y.; Saito, T.; Sawada, T.; Shimizu, H.; Strokovsky, E. A.; Sugaya, Y.; Suzuki, K.; Tokiyasu, A. O.; Tomioka, T.; Tsunemi, T.; Uchida, M.; Yorita, T.; LEPS Collaboration

2018-03-01

The differential cross sections and decay angular distributions for coherent ϕ -meson photoproduction from helium-4 are measured for the first time at forward angles with linearly polarized photons in the energy range Eγ=1.685 -2.385 GeV . Thanks to the target with spin-parity JP=0+ , unnatural-parity exchanges are absent, and thus natural-parity exchanges can be investigated clearly. The decay asymmetry with respect to photon polarization is shown to be very close to the maximal value. This ensures the strong dominance (>94 %) of natural-parity exchanges in this reaction. To evaluate the contribution from natural-parity exchanges to the forward cross section (θ =0∘ ) for the γ p →ϕ p reaction near threshold, the energy dependence of the forward cross section (θ =0∘ ) for the γ 4He →ϕ 4He reaction is analyzed. The comparison to γ p →ϕ p data suggests that enhancement of the forward cross section arising from natural-parity exchanges and/or destructive interference between natural-parity and unnatural-parity exchanges is needed in the γ p →ϕ p reaction near threshold.

The resonant structure of ^18Ne and its relevance in the breakout of the Hot CNO cycle

NASA Astrophysics Data System (ADS)

Almaraz-Calderon, S.; Tan, W.; Aprahamian, A.; Bucher, B.; Gorres, J.; Roberts, A.; Villano, A.; Wiescher, M.; Brune, C.; Heinen, Z.; Massey, T.; Mach, H.; Guray, N.; Guray, R. T.

2009-10-01

In explosive hydrogen burning environments such as Novae and X-ray bursts, temperatures and densities achieved are sufficiently high to bypass the beta decay of the waiting points of the hot CNO cycle by alpha captures, leading to a thermonuclear runaway via the rp-process. One of the two paths to a breakout from the hot CNO cycle is the route starting from ^14O(α,p)^17F followed by ^17F(p,γ)^18Ne and ^18Ne(α,p). The ^14O(α,p) reaction proceeds through resonant states in ^18Ne, making the reaction rate dependent on the excitation energies and spins as well as partial and total widths of these resonances. We used the ^16O(^3He,n) reaction and charged particle-neutron coincidences to measure the structure details of levels in ^18Ne. In particular, the α and proton decay branching ratios via ground state and excited states in ^17F were measured. The analysis of the data will allow us to provide crucial information to be included in the reaction network calculations that could have great impact on the nuclear energy generation and nucleosynthesis that occur in these explosive environments.

Measurement of the production of high-pT electrons from heavy-flavour hadron decays in Pb-Pb collisions at √{sNN} = 2.76 TeV

NASA Astrophysics Data System (ADS)

Adam, J.; Adamová, D.; Aggarwal, M. M.; Aglieri Rinella, G.; Agnello, M.; Agrawal, N.; Ahammed, Z.; Ahmad, S.; Ahn, S. U.; Aiola, S.; Akindinov, A.; Alam, S. N.; Albuquerque, D. S. D.; Aleksandrov, D.; Alessandro, B.; Alexandre, D.; Alfaro Molina, R.; Alici, A.; Alkin, A.; Alme, J.; Alt, T.; Altinpinar, S.; Altsybeev, I.; Alves Garcia Prado, C.; An, M.; Andrei, C.; Andrews, H. A.; Andronic, A.; Anguelov, V.; Anson, C.; Antičić, T.; Antinori, F.; Antonioli, P.; Anwar, R.; Aphecetche, L.; Appelshäuser, H.; Arcelli, S.; Arnaldi, R.; Arnold, O. W.; Arsene, I. C.; Arslandok, M.; Audurier, B.; Augustinus, A.; Averbeck, R.; Azmi, M. D.; Badalà, A.; Baek, Y. W.; Bagnasco, S.; Bailhache, R.; Bala, R.; Balasubramanian, S.; Baldisseri, A.; Baral, R. C.; Barbano, A. M.; Barbera, R.; Barile, F.; Barnaföldi, G. G.; Barnby, L. S.; Barret, V.; Bartalini, P.; Barth, K.; Bartke, J.; Bartsch, E.; Basile, M.; Bastid, N.; Basu, S.; Bathen, B.; Batigne, G.; Batista Camejo, A.; Batyunya, B.; Batzing, P. C.; Bearden, I. G.; Beck, H.; Bedda, C.; Behera, N. K.; Belikov, I.; Bellini, F.; Bello Martinez, H.; Bellwied, R.; Beltran, L. G. E.; Belyaev, V.; Bencedi, G.; Beole, S.; Bercuci, A.; Berdnikov, Y.; Berenyi, D.; Bertens, R. A.; Berzano, D.; Betev, L.; Bhasin, A.; Bhat, I. R.; Bhati, A. K.; Bhattacharjee, B.; Bhom, J.; Bianchi, L.; Bianchi, N.; Bianchin, C.; Bielčík, J.; Bielčíková, J.; Bilandzic, A.; Biro, G.; Biswas, R.; Biswas, S.; Bjelogrlic, S.; Blair, J. T.; Blau, D.; Blume, C.; Bock, F.; Bogdanov, A.; Boldizsár, L.; Bombara, M.; Bonora, M.; Book, J.; Borel, H.; Borissov, A.; Borri, M.; Botta, E.; Bourjau, C.; Braun-Munzinger, P.; Bregant, M.; Broker, T. A.; Browning, T. A.; Broz, M.; Brucken, E. J.; Bruna, E.; Bruno, G. E.; Budnikov, D.; Buesching, H.; Bufalino, S.; Buhler, P.; Buitron, S. A. I.; Buncic, P.; Busch, O.; Buthelezi, Z.; Butt, J. B.; Buxton, J. T.; Cabala, J.; Caffarri, D.; Caines, H.; Caliva, A.; Calvo Villar, E.; Camerini, P.; Carena, F.; Carena, W.; Carnesecchi, F.; Castillo Castellanos, J.; Castro, A. J.; Casula, E. A. R.; Ceballos Sanchez, C.; Cepila, J.; Cerello, P.; Cerkala, J.; Chang, B.; Chapeland, S.; Chartier, M.; Charvet, J. L.; Chattopadhyay, S.; Chattopadhyay, S.; Chauvin, A.; Chelnokov, V.; Cherney, M.; Cheshkov, C.; Cheynis, B.; Chibante Barroso, V.; Chinellato, D. D.; Cho, S.; Chochula, P.; Choi, K.; Chojnacki, M.; Choudhury, S.; Christakoglou, P.; Christensen, C. H.; Christiansen, P.; Chujo, T.; Chung, S. U.; Cicalo, C.; Cifarelli, L.; Cindolo, F.; Cleymans, J.; Colamaria, F.; Colella, D.; Collu, A.; Colocci, M.; Conesa Balbastre, G.; Conesa Del Valle, Z.; Connors, M. E.; Contreras, J. G.; Cormier, T. M.; Corrales Morales, Y.; Cortés Maldonado, I.; Cortese, P.; Cosentino, M. R.; Costa, F.; Crkovská, J.; Crochet, P.; Cruz Albino, R.; Cuautle, E.; Cunqueiro, L.; Dahms, T.; Dainese, A.; Danisch, M. C.; Danu, A.; Das, D.; Das, I.; Das, S.; Dash, A.; Dash, S.; de, S.; de Caro, A.; de Cataldo, G.; de Conti, C.; de Cuveland, J.; de Falco, A.; de Gruttola, D.; De Marco, N.; de Pasquale, S.; de Souza, R. D.; Deisting, A.; Deloff, A.; Deplano, C.; Dhankher, P.; di Bari, D.; di Mauro, A.; di Nezza, P.; di Ruzza, B.; Diaz Corchero, M. A.; Dietel, T.; Dillenseger, P.; Divià, R.; Djuvsland, Ø.; Dobrin, A.; Domenicis Gimenez, D.; Dönigus, B.; Dordic, O.; Drozhzhova, T.; Dubey, A. K.; Dubla, A.; Ducroux, L.; Duggal, A. K.; Dupieux, P.; Ehlers, R. J.; Elia, D.; Endress, E.; Engel, H.; Epple, E.; Erazmus, B.; Erhardt, F.; Espagnon, B.; Esumi, S.; Eulisse, G.; Eum, J.; Evans, D.; Evdokimov, S.; Eyyubova, G.; Fabbietti, L.; Fabris, D.; Faivre, J.; Fantoni, A.; Fasel, M.; Feldkamp, L.; Feliciello, A.; Feofilov, G.; Ferencei, J.; Fernández Téllez, A.; Ferreiro, E. G.; Ferretti, A.; Festanti, A.; Feuillard, V. J. G.; Figiel, J.; Figueredo, M. A. S.; Filchagin, S.; Finogeev, D.; Fionda, F. M.; Fiore, E. M.; Floris, M.; Foertsch, S.; Foka, P.; Fokin, S.; Fragiacomo, E.; Francescon, A.; Francisco, A.; Frankenfeld, U.; Fronze, G. G.; Fuchs, U.; Furget, C.; Furs, A.; Fusco Girard, M.; Gaardhøje, J. J.; Gagliardi, M.; Gago, A. M.; Gajdosova, K.; Gallio, M.; Galvan, C. D.; Gangadharan, D. R.; Ganoti, P.; Gao, C.; Garabatos, C.; Garcia-Solis, E.; Garg, K.; Garg, P.; Gargiulo, C.; Gasik, P.; Gauger, E. F.; Gay Ducati, M. B.; Germain, M.; Ghosh, P.; Ghosh, S. K.; Gianotti, P.; Giubellino, P.; Giubilato, P.; Gladysz-Dziadus, E.; Glässel, P.; Goméz Coral, D. M.; Gomez Ramirez, A.; Gonzalez, A. S.; Gonzalez, V.; González-Zamora, P.; Gorbunov, S.; Görlich, L.; Gotovac, S.; Grabski, V.; Graczykowski, L. K.; Graham, K. L.; Greiner, L.; Grelli, A.; Grigoras, C.; Grigoriev, V.; Grigoryan, A.; Grigoryan, S.; Grion, N.; Gronefeld, J. M.; Grosse-Oetringhaus, J. F.; Grosso, R.; Gruber, L.; Guber, F.; Guernane, R.; Guerzoni, B.; Gulbrandsen, K.; Gunji, T.; Gupta, A.; Gupta, R.; Guzman, I. B.; Haake, R.; Hadjidakis, C.; Hamagaki, H.; Hamar, G.; Hamon, J. C.; Harris, J. W.; Harton, A.; Hatzifotiadou, D.; Hayashi, S.; Heckel, S. T.; Hellbär, E.; Helstrup, H.; Herghelegiu, A.; Herrera Corral, G.; Herrmann, F.; Hess, B. A.; Hetland, K. F.; Hillemanns, H.; Hippolyte, B.; Hladky, J.; Horak, D.; Hosokawa, R.; Hristov, P.; Hughes, C.; Humanic, T. J.; Hussain, N.; Hussain, T.; Hutter, D.; Hwang, D. S.; Ilkaev, R.; Inaba, M.; Ippolitov, M.; Irfan, M.; Isakov, V.; Islam, M. S.; Ivanov, M.; Ivanov, V.; Izucheev, V.; Jacak, B.; Jacazio, N.; Jacobs, P. M.; Jadhav, M. B.; Jadlovska, S.; Jadlovsky, J.; Jahnke, C.; Jakubowska, M. J.; Janik, M. A.; Jayarathna, P. H. S. Y.; Jena, C.; Jena, S.; Jimenez Bustamante, R. T.; Jones, P. G.; Jusko, A.; Kalinak, P.; Kalweit, A.; Kang, J. H.; Kaplin, V.; Kar, S.; Karasu Uysal, A.; Karavichev, O.; Karavicheva, T.; Karayan, L.; Karpechev, E.; Kebschull, U.; Keidel, R.; Keijdener, D. L. D.; Keil, M.; Mohisin Khan, M.; Khan, P.; Khan, S. A.; Khanzadeev, A.; Kharlov, Y.; Khatun, A.; Khuntia, A.; Kileng, B.; Kim, D. W.; Kim, D. J.; Kim, D.; Kim, H.; Kim, J. S.; Kim, J.; Kim, M.; Kim, M.; Kim, S.; Kim, T.; Kirsch, S.; Kisel, I.; Kiselev, S.; Kisiel, A.; Kiss, G.; Klay, J. L.; Klein, C.; Klein, J.; Klein-Bösing, C.; Klewin, S.; Kluge, A.; Knichel, M. L.; Knospe, A. G.; Kobdaj, C.; Kofarago, M.; Kollegger, T.; Kolojvari, A.; Kondratiev, V.; Kondratyeva, N.; Kondratyuk, E.; Konevskikh, A.; Kopcik, M.; Kour, M.; Kouzinopoulos, C.; Kovalenko, O.; Kovalenko, V.; Kowalski, M.; Koyithatta Meethaleveedu, G.; Králik, I.; Kravčáková, A.; Krivda, M.; Krizek, F.; Kryshen, E.; Krzewicki, M.; Kubera, A. M.; Kučera, V.; Kuhn, C.; Kuijer, P. G.; Kumar, A.; Kumar, J.; Kumar, L.; Kumar, S.; Kundu, S.; Kurashvili, P.; Kurepin, A.; Kurepin, A. B.; Kuryakin, A.; Kushpil, S.; Kweon, M. J.; Kwon, Y.; La Pointe, S. L.; La Rocca, P.; Lagana Fernandes, C.; Lakomov, I.; Langoy, R.; Lapidus, K.; Lara, C.; Lardeux, A.; Lattuca, A.; Laudi, E.; Lazaridis, L.; Lea, R.; Leardini, L.; Lee, S.; Lehas, F.; Lehner, S.; Lehrbach, J.; Lemmon, R. C.; Lenti, V.; Leogrande, E.; León Monzón, I.; Lévai, P.; Li, S.; Li, X.; Lien, J.; Lietava, R.; Lindal, S.; Lindenstruth, V.; Lippmann, C.; Lisa, M. A.; Ljunggren, H. M.; Llope, W.; Lodato, D. F.; Loenne, P. I.; Loginov, V.; Loizides, C.; Lopez, X.; López Torres, E.; Lowe, A.; Luettig, P.; Lunardon, M.; Luparello, G.; Lupi, M.; Lutz, T. H.; Maevskaya, A.; Mager, M.; Mahajan, S.; Mahmood, S. M.; Maire, A.; Majka, R. D.; Malaev, M.; Maldonado Cervantes, I.; Malinina, L.; Mal'Kevich, D.; Malzacher, P.; Mamonov, A.; Manko, V.; Manso, F.; Manzari, V.; Mao, Y.; Marchisone, M.; Mareš, J.; Margagliotti, G. V.; Margotti, A.; Margutti, J.; Marín, A.; Markert, C.; Marquard, M.; Martin, N. A.; Martinengo, P.; Martínez, M. I.; Martínez García, G.; Martinez Pedreira, M.; Mas, A.; Masciocchi, S.; Masera, M.; Masoni, A.; Mastroserio, A.; Matyja, A.; Mayer, C.; Mazer, J.; Mazzilli, M.; Mazzoni, M. A.; Meddi, F.; Melikyan, Y.; Menchaca-Rocha, A.; Meninno, E.; Mercado Pérez, J.; Meres, M.; Mhlanga, S.; Miake, Y.; Mieskolainen, M. M.; Mikhaylov, K.; Milano, L.; Milosevic, J.; Mischke, A.; Mishra, A. N.; Mishra, T.; Miśkowiec, D.; Mitra, J.; Mitu, C. M.; Mohammadi, N.; Mohanty, B.; Molnar, L.; Montes, E.; Moreira de Godoy, D. A.; Moreno, L. A. P.; Moretto, S.; Morreale, A.; Morsch, A.; Muccifora, V.; Mudnic, E.; Mühlheim, D.; Muhuri, S.; Mukherjee, M.; Mulligan, J. D.; Munhoz, M. G.; Münning, K.; Munzer, R. H.; Murakami, H.; Murray, S.; Musa, L.; Musinsky, J.; Myers, C. J.; Naik, B.; Nair, R.; Nandi, B. K.; Nania, R.; Nappi, E.; Naru, M. U.; Natal da Luz, H.; Nattrass, C.; Navarro, S. R.; Nayak, K.; Nayak, R.; Nayak, T. K.; Nazarenko, S.; Nedosekin, A.; Negrao de Oliveira, R. A.; Nellen, L.; Ng, F.; Nicassio, M.; Niculescu, M.; Niedziela, J.; Nielsen, B. S.; Nikolaev, S.; Nikulin, S.; Nikulin, V.; Noferini, F.; Nomokonov, P.; Nooren, G.; Noris, J. C. C.; Norman, J.; Nyanin, A.; Nystrand, J.; Oeschler, H.; Oh, S.; Ohlson, A.; Okubo, T.; Olah, L.; Oleniacz, J.; Oliveira da Silva, A. C.; Oliver, M. H.; Onderwaater, J.; Oppedisano, C.; Orava, R.; Oravec, M.; Ortiz Velasquez, A.; Oskarsson, A.; Otwinowski, J.; Oyama, K.; Ozdemir, M.; Pachmayer, Y.; Pacik, V.; Pagano, D.; Pagano, P.; Paić, G.; Pal, S. K.; Palni, P.; Pan, J.; Pandey, A. K.; Papikyan, V.; Pappalardo, G. S.; Pareek, P.; Park, J.; Park, W. J.; Parmar, S.; Passfeld, A.; Paticchio, V.; Patra, R. N.; Paul, B.; Pei, H.; Peitzmann, T.; Peng, X.; Pereira da Costa, H.; Peresunko, D.; Perez Lezama, E.; Peskov, V.; Pestov, Y.; Petráček, V.; Petrov, V.; Petrovici, M.; Petta, C.; Piano, S.; Pikna, M.; Pillot, P.; Pimentel, L. O. D. L.; Pinazza, O.; Pinsky, L.; Piyarathna, D. B.; Płoskoń, M.; Planinic, M.; Pluta, J.; Pochybova, S.; Podesta-Lerma, P. L. M.; Poghosyan, M. G.; Polichtchouk, B.; Poljak, N.; Poonsawat, W.; Pop, A.; Poppenborg, H.; Porteboeuf-Houssais, S.; Porter, J.; Pospisil, J.; Pozdniakov, V.; Prasad, S. K.; Preghenella, R.; Prino, F.; Pruneau, C. A.; Pshenichnov, I.; Puccio, M.; Puddu, G.; Pujahari, P.; Punin, V.; Putschke, J.; Qvigstad, H.; Rachevski, A.; Raha, S.; Rajput, S.; Rak, J.; Rakotozafindrabe, A.; Ramello, L.; Rami, F.; Rana, D. B.; Raniwala, R.; Raniwala, S.; Räsänen, S. S.; Rascanu, B. T.; Rathee, D.; Ratza, V.; Ravasenga, I.; Read, K. F.; Redlich, K.; Rehman, A.; Reichelt, P.; Reidt, F.; Ren, X.; Renfordt, R.; Reolon, A. R.; Reshetin, A.; Reygers, K.; Riabov, V.; Ricci, R. A.; Richert, T.; Richter, M.; Riedler, P.; Riegler, W.; Riggi, F.; Ristea, C.; Rodríguez Cahuantzi, M.; Røed, K.; Rogochaya, E.; Rohr, D.; Röhrich, D.; Ronchetti, F.; Ronflette, L.; Rosnet, P.; Rossi, A.; Roukoutakis, F.; Roy, A.; Roy, C.; Roy, P.; Rubio Montero, A. J.; Rui, R.; Russo, R.; Ryabinkin, E.; Ryabov, Y.; Rybicki, A.; Saarinen, S.; Sadhu, S.; Sadovsky, S.; Šafařík, K.; Sahlmuller, B.; Sahoo, B.; Sahoo, P.; Sahoo, R.; Sahoo, S.; Sahu, P. K.; Saini, J.; Sakai, S.; Saleh, M. A.; Salzwedel, J.; Sambyal, S.; Samsonov, V.; Sandoval, A.; Sano, M.; Sarkar, D.; Sarkar, N.; Sarma, P.; Sas, M. H. P.; Scapparone, E.; Scarlassara, F.; Scharenberg, R. P.; Schiaua, C.; Schicker, R.; Schmidt, C.; Schmidt, H. R.; Schmidt, M.; Schukraft, J.; Schutz, Y.; Schwarz, K.; Schweda, K.; Scioli, G.; Scomparin, E.; Scott, R.; Šefčík, M.; Seger, J. E.; Sekiguchi, Y.; Sekihata, D.; Selyuzhenkov, I.; Senosi, K.; Senyukov, S.; Serradilla, E.; Sett, P.; Sevcenco, A.; Shabanov, A.; Shabetai, A.; Shadura, O.; Shahoyan, R.; Shangaraev, A.; Sharma, A.; Sharma, A.; Sharma, M.; Sharma, M.; Sharma, N.; Sheikh, A. I.; Shigaki, K.; Shou, Q.; Shtejer, K.; Sibiriak, Y.; Siddhanta, S.; Sielewicz, K. M.; Siemiarczuk, T.; Silvermyr, D.; Silvestre, C.; Simatovic, G.; Simonetti, G.; Singaraju, R.; Singh, R.; Singhal, V.; Sinha, T.; Sitar, B.; Sitta, M.; Skaali, T. B.; Slupecki, M.; Smirnov, N.; Snellings, R. J. M.; Snellman, T. W.; Song, J.; Song, M.; Song, Z.; Soramel, F.; Sorensen, S.; Sozzi, F.; Spiriti, E.; Sputowska, I.; Srivastava, B. K.; Stachel, J.; Stan, I.; Stankus, P.; Stenlund, E.; Steyn, G.; Stiller, J. H.; Stocco, D.; Strmen, P.; Suaide, A. A. P.; Sugitate, T.; Suire, C.; Suleymanov, M.; Suljic, M.; Sultanov, R.; Šumbera, M.; Sumowidagdo, S.; Suzuki, K.; Swain, S.; Szabo, A.; Szarka, I.; Szczepankiewicz, A.; Szymanski, M.; Tabassam, U.; Takahashi, J.; Tambave, G. J.; Tanaka, N.; Tarhini, M.; Tariq, M.; Tarzila, M. G.; Tauro, A.; Tejeda Muñoz, G.; Telesca, A.; Terasaki, K.; Terrevoli, C.; Teyssier, B.; Thakur, D.; Thomas, D.; Tieulent, R.; Tikhonov, A.; Timmins, A. R.; Toia, A.; Tripathy, S.; Trogolo, S.; Trombetta, G.; Trubnikov, V.; Trzaska, W. H.; Tsuji, T.; Tumkin, A.; Turrisi, R.; Tveter, T. S.; Ullaland, K.; Umaka, E. N.; Uras, A.; Usai, G. L.; Utrobicic, A.; Vala, M.; van der Maarel, J.; van Hoorne, J. W.; van Leeuwen, M.; Vanat, T.; Vande Vyvre, P.; Varga, D.; Vargas, A.; Vargyas, M.; Varma, R.; Vasileiou, M.; Vasiliev, A.; Vauthier, A.; Vázquez Doce, O.; Vechernin, V.; Veen, A. M.; Velure, A.; Vercellin, E.; Vergara Limón, S.; Vernet, R.; Vértesi, R.; Vickovic, L.; Vigolo, S.; Viinikainen, J.; Vilakazi, Z.; Villalobos Baillie, O.; Villatoro Tello, A.; Vinogradov, A.; Vinogradov, L.; Virgili, T.; Vislavicius, V.; Vodopyanov, A.; Völkl, M. A.; Voloshin, K.; Voloshin, S. A.; Volpe, G.; von Haller, B.; Vorobyev, I.; Voscek, D.; Vranic, D.; Vrláková, J.; Wagner, B.; Wagner, J.; Wang, H.; Wang, M.; Watanabe, D.; Watanabe, Y.; Weber, M.; Weber, S. G.; Weiser, D. F.; Wessels, J. P.; Westerhoff, U.; Whitehead, A. M.; Wiechula, J.; Wikne, J.; Wilk, G.; Wilkinson, J.; Willems, G. A.; Williams, M. C. S.; Windelband, B.; Winn, M.; Witt, W. E.; Yalcin, S.; Yang, P.; Yano, S.; Yin, Z.; Yokoyama, H.; Yoo, I.-K.; Yoon, J. H.; Yurchenko, V.; Zaccolo, V.; Zaman, A.; Zampolli, C.; Zanoli, H. J. C.; Zaporozhets, S.; Zardoshti, N.; Zarochentsev, A.; Závada, P.; Zaviyalov, N.; Zbroszczyk, H.; Zhalov, M.; Zhang, H.; Zhang, X.; Zhang, Y.; Zhang, C.; Zhang, Z.; Zhao, C.; Zhigareva, N.; Zhou, D.; Zhou, Y.; Zhou, Z.; Zhu, H.; Zhu, J.; Zichichi, A.; Zimmermann, A.; Zimmermann, M. B.; Zinovjev, G.; Zmeskal, J.; Alice Collaboration

2017-08-01

Electrons from heavy-flavour hadron decays (charm and beauty) were measured with the ALICE detector in Pb-Pb collisions at a centre-of-mass of energy √{sNN} = 2.76 TeV. The transverse momentum (pT) differential production yields at mid-rapidity were used to calculate the nuclear modification factor RAA in the interval 3

Beta Decay Half-Life of 84Mo

NASA Astrophysics Data System (ADS)

Stoker, J. B.; Mantica, P. F.; Bazin, D.; Bickley, A.; Becerril, A.; Crawford, H.; Cruse, K.; Estrade, A.; Mosby, M.; Guess, C. J.; Hitt, G. W.; Lorusso, G.; Matos, M.; Meharchand, R.; Minamisono, K.; Montes, F.; Pereira, J.; Perdikakis, G.; Pinter, J. S.; Schatz, H.; Vredevoogd, J.; Zegers, R. G. T.

2008-10-01

The β-decay half-life ^84Mo governs leakage out of the Zr-Nb cycle, a high temperature rp-process endpoint in x-ray binaries [1]. Treatment of the background and the poor statistics accumulated during the previous half-life measurement leave questions about statistical and systematic errors. We have remeasured the half-life of ^84Mo using a concerted setup of the NSCL β-Counting System [3] and 16 detectors from the Segmented Germanium Array [4]. We will report the half-life for ^84Mo, deduced using 40 times the previous sample size. The application of the NSCL RF Fragment Separator to remove unwanted isotopes, and hence reduce background for the half-life measurement, will also be discussed. [1] H. Schatz et al., Phys. Rep. 294, 167 1998 [2] P. Kienle et al., Prog. Part. Nuc. Phys. 46, 73 2001 [3] J. Prisciandaro et al., NIM A 505, 140 2003 [4] W. Mueller et al., NIM A 466, 492 2001 [5] D. Gorelov et al. PAC 2005, Knoxville, TN, May 16-20

Early ⁵⁶Ni decay gamma rays from SN2014J suggest an unusual explosion.

PubMed

Diehl, Roland; Siegert, Thomas; Hillebrandt, Wolfgang; Grebenev, Sergei A; Greiner, Jochen; Krause, Martin; Kromer, Markus; Maeda, Keiichi; Röpke, Friedrich; Taubenberger, Stefan

2014-09-05

Type Ia supernovae result from binary systems that include a carbon-oxygen white dwarf, and these thermonuclear explosions typically produce 0.5 solar mass of radioactive (56)Ni. The (56)Ni is commonly believed to be buried deeply in the expanding supernova cloud. In SN2014J, we detected the lines at 158 and 812 kiloelectron volts from (56)Ni decay (time ~8.8 days) earlier than the expected several-week time scale, only ~20 days after the explosion and with flux levels corresponding to roughly 10% of the total expected amount of (56)Ni. Some mechanism must break the spherical symmetry of the supernova and at the same time create a major amount of (56)Ni at the outskirts. A plausible explanation is that a belt of helium from the companion star is accreted by the white dwarf, where this material explodes and then triggers the supernova event. Copyright © 2014, American Association for the Advancement of Science.

Delayed fission and multifragmentation in sub-keV C60 - Au(0 0 1) collisions via molecular dynamics simulations: Mass distributions and activated statistical decay

NASA Astrophysics Data System (ADS)

Bernstein, V.; Kolodney, E.

2017-10-01

We have recently observed, both experimentally and computationally, the phenomenon of postcollision multifragmentation in sub-keV surface collisions of a C60 projectile. Namely, delayed multiparticle breakup of a strongly impact deformed and vibrationally excited large cluster collider into several large fragments, after leaving the surface. Molecular dynamics simulations with extensive statistics revealed a nearly simultaneous event, within a sub-psec time window. Here we study, computationally, additional essential aspects of this new delayed collisional fragmentation which were not addressed before. Specifically, we study here the delayed (binary) fission channel for different impact energies both by calculating mass distributions over all fission events and by calculating and analyzing lifetime distributions of the scattered projectile. We observe an asymmetric fission resulting in a most probable fission channel and we find an activated exponential (statistical) decay. Finally, we also calculate and discuss the fragment mass distribution in (triple) multifragmentation over different time windows, in terms of most abundant fragments.

Application of PIXE in the determination of the production cross section of a radionuclide decaying by electron capture

NASA Astrophysics Data System (ADS)

Morales, J. R.; Chesta, M. A.; Cancino, S. A.; Miranda, P. A.; Dinator, M. I.; Avila, M. J.

2005-01-01

Proton induced X-ray emission (PIXE) has been applied to the measurement of the production cross section of a radionuclide decaying by electron capture. By performing a PIXE type experiment on the daughter nuclide important advantages are obtained. The determination of some factors with usually large uncertainties, like solid angle and detector efficiency were avoided. The method was applied to the determination of cross section of the reaction 63Cu(d, p)64Cu at 2.4 MeV for 64Cu production. This result is in full agreement with that obtained through the decay of the 1346 keV gamma ray of 64Cu.

Two-neutron sequential decay of O 24

DOE PAGES

Jones, M. D.; Frank, N.; Baumann, T.; ...

2015-11-25

In this study, a two-neutron unbound excited state of 24O was populated through a (d,d') reaction at 83.4 MeV/nucleon. A state at E=715±110 (stat) ±45 (sys) keV with a width of Γ<2 MeV was observed above the two-neutron separation energy placing it at 7.65 ± 0.2 MeV with respect to the ground state. Three-body correlations for the decay of 24O → 22O + 2n show clear evidence for a sequential decay through an intermediate state in 23O. Neither a di-neutron nor phase-space model for the three-body breakup were able to describe these correlations.

Two-neutron sequential decay of O 24

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jones, M. D.; Frank, N.; Baumann, T.

In this study, a two-neutron unbound excited state of 24O was populated through a (d,d') reaction at 83.4 MeV/nucleon. A state at E=715±110 (stat) ±45 (sys) keV with a width of Γ<2 MeV was observed above the two-neutron separation energy placing it at 7.65 ± 0.2 MeV with respect to the ground state. Three-body correlations for the decay of 24O → 22O + 2n show clear evidence for a sequential decay through an intermediate state in 23O. Neither a di-neutron nor phase-space model for the three-body breakup were able to describe these correlations.

Change of nuclear configurations in the neutrinoless double-β decay of 130Te →130Be and 136Xe136Ba

NASA Astrophysics Data System (ADS)

Entwisle, J. P.; Kay, B. P.; Tamii, A.; Adachi, S.; Aoi, N.; Clark, J. A.; Freeman, S. J.; Fujita, H.; Fujita, Y.; Furuno, T.; Hashimoto, T.; Hoffman, C. R.; Ideguchi, E.; Ito, T.; Iwamoto, C.; Kawabata, T.; Liu, B.; Miura, M.; Ong, H. J.; Schiffer, J. P.; Sharp, D. K.; Süsoy, G.; Suzuki, T.; Szwec, S. V.; Takaki, M.; Tsumura, M.; Yamamoto, T.

2016-06-01

The change in the configuration of valence protons between the initial and final states in the neutrinoless double-β decay of 130Te → 130Be and of 136Xe136Ba has been determined by measuring the cross sections of the (d ,3He) reaction with 101-MeV deuterons. Together with our recent determination of the relevant neutron configurations involved in the process, a quantitative comparison with the latest shell-model and interacting-boson-model calculations reveals significant discrepancies. These are the same calculations used to determine the nuclear matrix elements governing the rate of neutrinoless double-β decay in these systems.

Change of Nuclear Configurations in the Neutrinoless Double-β Decay of 130Te → 130Xe and 136Xe → 136Ba

DOE PAGES

Entwisle, J. P.; Kay, B. P.; Tamii, A.; ...

2016-06-13

The change in the configuration of valence protons between the initial and final states in the neutrinoless double-beta decay of Te-130 -> Xe-130 and of Xe-136 -> Ba-136 has been determined by measuring the cross sections of the (d,He-3) reaction with 101-MeV deuterons. Together with our recent determination of the relevant neutron configurations involved in the process, a quantitative comparison with the latest shell-model and interacting-boson-model calculations reveals significant discrepancies. These are the same calculations used to determine the nuclear matrix elements governing the rate of neutrinoless double-beta decay in these systems.

Elastic and Inelastic Scattering of Neutrons from Neon and Argon: Impact on Neutrinoless Double-Beta Decay and Dark Matter Experimental Programs

NASA Astrophysics Data System (ADS)

MacMullin, Sean Patrick

In underground physics experiments, such as neutrinoless double-beta decay and dark matter searches, fast neutrons may be the dominant and potentially irreducible source of background. Experimental data for the elastic and inelastic scattering cross sections of neutrons from argon and neon, which are target and shielding materials of interest to the dark matter and neutrinoless double-beta decay communities, were previously unavailable. Unmeasured neutron scattering cross sections are often accounted for incorrectly in Monte-Carlo simulations. Elastic scattering cross sections were measured at the Triangle Universities Nuclear Laboratory (TUNL) using the neutron time-of-flight technique. Angular distributions for neon were measured at 5.0 and 8.0 MeV. One full angular distribution was measured for argon at 6.0 MeV. The cross-section data were compared to calculations using a global optical model. Data were also fit using the spherical optical model. These model fits were used to predict the elastic scattering cross section at unmeasured energies and also provide a benchmark where the global optical models are not well constrained. Partial gamma-ray production cross sections for (n,xngamma ) reactions in natural argon and neon were measured using the broad spectrum neutron beam at the Los Alamos Neutron Science Center (LANSCE). Neutron energies were determined using time of flight and resulting gamma rays from neutron-induced reactions were detected using the GErmanium Array for Neutron Induced Excitations (GEANIE). Partial gamma-ray production cross sections for six transitions in 40Ar, two transitions in 39Ar and the first excited state transitions is 20Ne and 22Ne were measured from threshold to a neutron energy where the gamma-ray yield dropped below the detection sensitivity. Measured (n,xngamma) cross sections were compared with calculations using the TALYS and CoH3 nuclear reaction codes. These new measurements will help to identify potential backgrounds in neutrinoless double-beta decay and dark matter experiments that use argon or neon. The measurements will also aid in the identification of neutron interactions in these experiments through the detection of gamma rays produced by ( n,xngamma) reactions.

Modification of the nanostructure of lignocellulose cell walls via a non-enzymatic lignocellulose deconstruction system in brown rot wood-decay fungi.

PubMed

Goodell, Barry; Zhu, Yuan; Kim, Seong; Kafle, Kabindra; Eastwood, Daniel; Daniel, Geoffrey; Jellison, Jody; Yoshida, Makoto; Groom, Leslie; Pingali, Sai Venkatesh; O'Neill, Hugh

2017-01-01

Wood decayed by brown rot fungi and wood treated with the chelator-mediated Fenton (CMF) reaction, either alone or together with a cellulose enzyme cocktail, was analyzed by small angle neutron scattering (SANS), sum frequency generation (SFG) spectroscopy, Fourier transform infrared (FTIR) analysis, X-ray diffraction (XRD), atomic force microscopy (AFM), and transmission electron microscopy (TEM). Results showed that the CMF mechanism mimicked brown rot fungal attack for both holocellulose and lignin components of the wood. Crystalline cellulose and lignin were both depolymerized by the CMF reaction. Porosity of the softwood cell wall did not increase during CMF treatment, enzymes secreted by the fungi did not penetrate the decayed wood. The enzymes in the cellulose cocktail also did not appear to alter the effects of the CMF-treated wood relative to enhancing cell wall deconstruction. This suggests a rethinking of current brown rot decay models and supports a model where monomeric sugars and oligosaccharides diffuse from the softwood cell walls during non-enzymatic action. In this regard, the CMF mechanism should not be thought of as a "pretreatment" used to permit enzymatic penetration into softwood cell walls, but instead it enhances polysaccharide components diffusing to fungal enzymes located in wood cell lumen environments during decay. SANS and other data are consistent with a model for repolymerization and aggregation of at least some portion of the lignin within the cell wall, and this is supported by AFM and TEM data. The data suggest that new approaches for conversion of wood substrates to platform chemicals in biorefineries could be achieved using the CMF mechanism with >75% solubilization of lignocellulose, but that a more selective suite of enzymes and other downstream treatments may be required to work when using CMF deconstruction technology. Strategies to enhance polysaccharide release from lignocellulose substrates for enhanced enzymatic action and fermentation of the released fraction would also aid in the efficient recovery of the more uniform modified lignin fraction that the CMF reaction generates to enhance biorefinery profitability.

X-Ray Burst Oscillations: From Flame Spreading to the Cooling Wake

NASA Technical Reports Server (NTRS)

Mahmoodifar, Simin; Strohmayer, Tod

2016-01-01

Type I X-ray bursts are thermonuclear flashes observed from the surfaces of accreting neutron stars (NSs) in low mass X-ray binaries. Oscillations have been observed during the rise and/or decay of some of these X-ray bursts. Those seen during the rise can be well explained by a spreading hot spot model, but large amplitude oscillations in the decay phase remain mysterious because of the absence of a clear-cut source of asymmetry. To date there have not been any quantitative studies that consistently track the oscillation amplitude both during the rise and decay (cooling tail) of bursts. Here we compute the light curves and amplitudes of oscillations in X-ray burst models that realistically account for both flame spreading and subsequent cooling. We present results for several such "cooling wake" models, a "canonical" cooling model where each patch on the NS surface heats and cools identically, or with a latitude-dependent cooling timescale set by the local effective gravity, and an "asymmetric" model where parts of the star cool at significantly different rates. We show that while the canonical cooling models can generate oscillations in the tails of bursts, they cannot easily produce the highest observed modulation amplitudes. Alternatively, a simple phenomenological model with asymmetric cooling can achieve higher amplitudes consistent with the observations.

Normal mode analysis on the relaxation of an excited nitromethane molecule in argon bath

NASA Astrophysics Data System (ADS)

Rivera-Rivera, Luis; Wagner, Albert

In our previous work [J. Chem. Phys. 142, 014303 (2015)] classical molecular dynamics simulations followed in an Ar bath the relaxation of nitromethane (CH3NO2) instantaneously excited by statistically distributing 50 kcal/mol among all its internal degrees of freedom. The 300 K Ar bath was at pressures of 10 to 400 atm, a range spanning the breakdown of the isolated binary collision approximation. Both rotational and vibrational energies exhibit multi-exponential decay. This study explores mode-specific mechanisms at work in the decay process. With the separation of rotation and vibration developed by Rhee and Kim [J. Chem. Phys. 107, 1394 (1997)], one can show that the vibrational kinetic energy decomposes only into vibrational normal modes while the rotational and Coriolis energies decompose into both vibrational and rotational normal modes. Then the saved CH3NO2 positions and momenta can be converted into mode-specific energies whose decay over 1000 ps can be monitored. The results identify vibrational and rotational modes that promote/resist energy lost and drive multi-exponential behavior. Increasing pressure can be shown to increasingly interfere with post-collision IVR. The work was supported by the U.S. Department of Energy, Office of Science, Chemical Sciences, Geosciences, and Biosciences Division.

Short range shooting distance estimation using variable pressure SEM images of the surroundings of bullet holes in textiles.

PubMed

Hinrichs, Ruth; Frank, Paulo Ricardo Ost; Vasconcellos, M A Z

2017-03-01

Modifications of cotton and polyester textiles due to shots fired at short range were analyzed with a variable pressure scanning electron microscope (VP-SEM). Different mechanisms of fiber rupture as a function of fiber type and shooting distance were detected, namely fusing, melting, scorching, and mechanical breakage. To estimate the firing distance, the approximately exponential decay of GSR coverage as a function of radial distance from the entrance hole was determined from image analysis, instead of relying on chemical analysis with EDX, which is problematic in the VP-SEM. A set of backscattered electron images, with sufficient magnification to discriminate micrometer wide GSR particles, was acquired at different radial distances from the entrance hole. The atomic number contrast between the GSR particles and the organic fibers allowed to find a robust procedure to segment the micrographs into binary images, in which the white pixel count was attributed to GSR coverage. The decrease of the white pixel count followed an exponential decay, and it was found that the reciprocal of the decay constant, obtained from the least-square fitting of the coverage data, showed a linear dependence on the shooting distance. Copyright © 2017 Elsevier Ireland Ltd. All rights reserved.

Recent Results on SNRs and PWNe from the Fermi Large Area Telescope

NASA Technical Reports Server (NTRS)

Hays, Elizabeth

2010-01-01

a) Symbiotic Binary System: White dwarf + red giant system. b) Nova: White dwarf builds up mass envelope to the point of thermonuclear fusion. c) Dramatic increase in visual magnitude. d) Recurrent Nova? e) Hints but no strong confirmation of previous nova f) Pre-nova activity: 1) White dwarf shows ongoing variability at level of several in magnitude. 2) V407 Cyg companion is a Mira star showing variability at level of several in magnitude. g) Origin of the gamma rays? 1) Strong shock propagating into dense medium around giant star land stellar wind. 2) Pion decay or electron processes?

[Analysis of carbon balance and study on mechanism in anoxic-oxic-settling-anaerobic sludge reduction process].

PubMed

Zhai, Xiao-Min; Gao, Xu; Zhang, Man-Man; Jia, Li; Guo, Jin-Song

2012-07-01

In order to deeply explore the mechanism of sludge reduction in OSA system, carbon balance was performed in an anoxic-oxic-settling-anaerobic (A + OSA) system and a reference AO system to investigate effects of inserting a sludge holding tank in sludge cycle line on the sludge reduction process. Meanwhile, carbon mass change in each reaction unit was identified in terms of solid, liquid and gas phases. The causes of excess sludge reduction in A + OSA system were deduced. The carbon balance results show that when the hydraulic retention time in the sludge holding tank is 7.14 h, carbon percent in solid phase of the sludge reduction system is nearly 50% higher than that of the reference system, supporting the consequence that sludge reduction rate of 49.98% had been achieved. The insertion of a sludge holding tank in the sludge return circuit can be effective in sludge reduction. Carbon changes in each unit reveal that the amount of carbon consumed for biosynthesis in the anoxic and oxic tanks (main reaction zone) of the sludge reduction system is higher than in that of the reference system. Sludge decay is observed in the sludge holding tank. Furthermore, CH4 released from the sludge holding tank is significantly higher than that from the main reaction zone. The DGGE profiles show that there are hydrolytic-fermentative bacteria in the sludge holding tank related to sludge decay. The excess sludge reduction in the A + OSA system could be a result of the combination of sludge decay in the sludge holding tank and sludge compensatory growth in the main reaction cell.

Plasmon-driven sequential chemical reactions in an aqueous environment.

PubMed

Zhang, Xin; Wang, Peijie; Zhang, Zhenglong; Fang, Yurui; Sun, Mengtao

2014-06-24

Plasmon-driven sequential chemical reactions were successfully realized in an aqueous environment. In an electrochemical environment, sequential chemical reactions were driven by an applied potential and laser irradiation. Furthermore, the rate of the chemical reaction was controlled via pH, which provides indirect evidence that the hot electrons generated from plasmon decay play an important role in plasmon-driven chemical reactions. In acidic conditions, the hot electrons were captured by the abundant H(+) in the aqueous environment, which prevented the chemical reaction. The developed plasmon-driven chemical reactions in an aqueous environment will significantly expand the applications of plasmon chemistry and may provide a promising avenue for green chemistry using plasmon catalysis in aqueous environments under irradiation by sunlight.

Plasmon-driven sequential chemical reactions in an aqueous environment

PubMed Central

Zhang, Xin; Wang, Peijie; Zhang, Zhenglong; Fang, Yurui; Sun, Mengtao

2014-01-01

Plasmon-driven sequential chemical reactions were successfully realized in an aqueous environment. In an electrochemical environment, sequential chemical reactions were driven by an applied potential and laser irradiation. Furthermore, the rate of the chemical reaction was controlled via pH, which provides indirect evidence that the hot electrons generated from plasmon decay play an important role in plasmon-driven chemical reactions. In acidic conditions, the hot electrons were captured by the abundant H+ in the aqueous environment, which prevented the chemical reaction. The developed plasmon-driven chemical reactions in an aqueous environment will significantly expand the applications of plasmon chemistry and may provide a promising avenue for green chemistry using plasmon catalysis in aqueous environments under irradiation by sunlight. PMID:24958029

Foundations of an effective-one-body model for coalescing binaries on eccentric orbits

NASA Astrophysics Data System (ADS)

Hinderer, Tanja; Babak, Stanislav

2017-11-01

We develop the foundations of an effective-one-body (EOB) model for eccentric binary coalescences that includes the conservative dynamics, radiation reaction, and gravitational waveform modes from the inspiral and the merger-ringdown signals. Our approach uses the strategy that is commonly employed in black-hole perturbation theory: we introduce an efficient, relativistic parameterization of the dynamics that is defined by the orbital geometry and consists of a set of phase variables and quantities that evolve only due to gravitational radiation reaction. Specializing to nonspinning binaries, we derive the EOB equations of motion for the new variables and make use of the fundamental frequencies of the motion to compute the binary's radiative multipole moments that determine the gravitational waves. Our treatment has several advantages over the quasi-Keplerian approach that is often used in post-Newtonian (PN) calculations: a smaller set of variables, parameters that reflect the features of strong-field dynamics, and a greater transparency of the calculations when using the fundamental frequencies that leads to simplifications and an unambiguous orbit-averaging operation. While our description of the conservative dynamics is fully relativistic, we limit explicit derivations in the radiative sector to 1.5PN order for simplicity. This already enables us to establish methods for computing both instantaneous and hereditary contributions to the gravitational radiation in EOB coordinates that have straightforward extensions to higher PN order. The weak-field, small eccentricity limit of our results for the orbit-averaged fluxes agrees with known PN results when expressed in terms of gauge-invariant quantities. We further address considerations for the numerical implementation of the model and the completion of the waveforms to include the merger and ringdown signals, and provide illustrative results.

On the Nature of the Variability Power Decay toward Soft Spectral States in X-Ray Binaries: Case Study in Cygnus X-1

NASA Astrophysics Data System (ADS)

Titarchuk, Lev; Shaposhnikov, Nikolai

2008-05-01

A characteristic feature of the Fourier power density spectrum (PDS) observed from black hole X-ray binaries in low/hard and intermediate spectral states is a broadband-limited noise characterized by a constant below some frequency (a "break" frequency) and a power law above this frequency. It has been shown that the variability of this type can be produced by the inward diffusion of the local driving perturbations in a bounded configuration (accretion disk or corona). In the framework of this model, the perturbation diffusion time t0 is related to the phenomenological break frequency, while the PDS power-law slope above the "break" is determined by the viscosity distribution over the configuration. The perturbation diffusion scenario explains the decay of the power of X-ray variability observed in a number of compact sources (containing black holes and neutron stars) during an evolution of these sources from low/hard to high/soft states. We compare the model predictions with the subset of data from Cyg X-1 collected by the Rossi X-Ray Time Explorer (RXTE). Our extensive analysis of the Cyg X-1 PDSs demonstrates that the observed integrated power Px decreases approximately as the square root of the characteristic frequency of the driving oscillations νdr. The RXTE observations of Cyg X-1 allow us to infer Pdr and t0 as a function of νdr. Using the inferred dependences of the integrated power of the driving oscillations Pdr and t0 on νdr we demonstrate that the power predicted by the model also decays as Px,diff propto ν-0.5dr, which is similar to the observed Px behavior. We also apply the basic parameters of observed PDSs, power-law indices, and low-frequency quasi-periodic oscillations to infer the Reynolds number (Re) from the observations using the method developed in our previous paper. Our analysis shows that Re increases from values of about 10 in low/hard state to about 70 during the high/soft state.

On the nature of the variability power decay towards soft spectral states in X-ray binaries. Case study in Cyg X-1

NASA Astrophysics Data System (ADS)

Titarchuk, Lev; Shaposhnikov, Nikolai

2008-01-01

A characteristic feature of the Fourier Power Density Spectrum (PDS) observed from black hole X-ray binaries in low/hard and intermediate spectral states is a broad band-limited noise, characterized by a constant below some frequency (a ``break'' frequency) and a power law above this frequency. It has been shown that the variability of this type can be produced by the inward diffusion of the local driving perturbations in a bounded configuration (accretion disk or corona). In the framework of this model, the perturbation diffusion time t0 is related to the phenomenological break frequency, while the PDS power-law slope above the ``break'' is determined by the viscosity distribution over the configuration. The perturbation diffusion scenario explains the decay of the power of X-ray variability observed in a number of compact sources (containing black hole and neutron star) during an evolution of theses sources from low/hard to high/soft states. We compare the model predictions with the subset of data from Cyg X-1 collected by the Rossi X-ray Time Explorer (RXTE). Our extensive analysis of the Cyg X-1 PDSs demonstrates that the observed integrated power Px decreases approximately as a square root of the characteristic frequency of the driving oscillations νdr. The RXTE observations of Cyg X-1 allow us to infer Pdr and t0 as a function of νdr. Using the inferred dependences of the integrated power of the driving oscillations Pdr and t0 on νdr we demonstrate that the power predicted by the model also decays as Px,diff~νdr-0.5 that is similar to the observed Px behavior. We also apply the basic parameters of observed PDSs, power-law index and low frequency quasiperiodic oscillations, to infer Reynolds (Re) number from the observations using the method developed in our previous paper. Our analysis shows that Re-number increases from values about 10 in low/hard state to that about 70 during the high/soft state.

Test and Evaluation Management Guide, Third Edition.

DTIC Science & Technology

1998-03-01

chemical tests — chemical mixing and biotoxicity . Chemical-mixing tests are con- ducted to obtain information on the binary chemical reaction... Biotoxicity tests are per- formed to assess the potency of the agent generated. Chemical weapons testing, of necessity, relies heavily on the use of non

A numerical treatment of radiative nanofluid 3D flow containing gyrotactic microorganism with anisotropic slip, binary chemical reaction and activation energy.

PubMed

Lu, Dianchen; Ramzan, M; Ullah, Naeem; Chung, Jae Dong; Farooq, Umer

2017-12-05

A numerical investigation of steady three dimensional nanofluid flow carrying effects of gyrotactic microorganism with anisotropic slip condition along a moving plate near a stagnation point is conducted. Additionally, influences of Arrhenius activation energy, joule heating accompanying binary chemical reaction and viscous dissipation are also taken into account. A system of nonlinear differential equations obtained from boundary layer partial differential equations is found by utilization of apposite transformations. RK fourth and fifth order technique of Maple software is engaged to acquire the solution of the mathematical model governing the presented fluid flow. A Comparison with previously done study is also made and a good agreement is achieved with existing results; hence reliable results are being presented. Evaluations are carried out for involved parameters graphically against velocity, temperature, concentration fields, microorganism distribution, density number, local Nusselt and Sherwood numbers. It is detected that microorganism distribution exhibit diminishing behavior for rising values of bio-convection Lewis and Peclet numbers.

Experimental investigation of the phase equilibria and thermodynamic assessment in the U-Ga and U-Al-Ga systems

NASA Astrophysics Data System (ADS)

Moussa, Chantal; Berche, Alexandre; Barbosa, José; Pasturel, Mathieu; Stepnik, Bertrand; Tougait, Olivier

2018-02-01

The phase relations in the binary U-Ga and ternary U-Al-Ga systems were established as an isopleth section and two isothermal sections at 900 K and 1150 K for the whole concentration range, respectively. They were experimentally determined by means of powder and single crystal XRD, SEM-EDS analyses on both as-cast and heat-treated samples and DTA measurements. Both systems were thermodynamically assessed using the Calphad method based on the available data, i.e. phase relations and thermodynamic properties. The new description of the U-Ga phase diagram improves the composition-temperature description for most of invariant reactions. The U-Al-Ga system is characterized by large ternary extensions of the binary phases and the absence of ternary intermediate phase at both 900 K and 1150 K. These experimental results are nicely reproduced by the Calphad assessment, allowing to extract the thermodynamic parameters further used to calculate the liquidus projection and the invariant reactions along with their temperature.

One-step hydrothermal synthesis of carboxyl-functionalized upconversion phosphors for bioapplications.

PubMed

Yang, Jianping; Shen, Dengke; Li, Xiaomin; Li, Wei; Fang, Yin; Wei, Yong; Yao, Chi; Tu, Bo; Zhang, Fan; Zhao, Dongyuan

2012-10-22

In this paper, we report a facile one-step hydrothermal method to synthesize phase-, size-, and shape-controlled carboxyl-functionalized rare-earth fluorescence upconversion phosphors by using a small-molecule binary acid, such as malonic acid, oxalic acid, succinic acid, or tartaric acid as capping agent. The crystals, from nano- to microstructures with diverse shapes that include nanospheres, microrods, hexagonal prisms, microtubes, microdisks, polygonal columns, and hexagonal tablets, can be obtained with different reaction times, reaction temperatures, molar ratios of capping agent to sodium hydroxide, and by varying the binary acids. Fourier transform infrared, thermogravimetric analysis, and upconversion luminescence spectra measurements indicate that the synthesized NaYF(4):Yb/Er products with hydrophilic carboxyl-functionalized surface offer efficient upconversion luminescent performance. Furthermore, the antibody/secondary antibody conjugation can be realized by the carboxyl-functionalized surfaces of the upconversion phosphors, thus indicating the potential bioapplications of these kinds of materials. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

A small organic compound enhances the religation reaction of human topoisomerase I and identifies crucial elements for the religation mechanism

PubMed Central

Arnò, Barbara; Coletta, Andrea; Tesauro, Cinzia; Zuccaro, Laura; Fiorani, Paola; Lentini, Sara; Galloni, Pierluca; Conte, Valeria; Floris, Barbara; Desideri, Alessandro

2013-01-01

The different steps of the human Top1 (topoisomerase I) catalytic cycle have been analysed in the presence of a pentacyclic-diquinoid synthetic compound. The experiments indicate that it efficiently inhibits the cleavage step of the enzyme reaction, fitting well into the catalytic site. Surprisingly the compound, when incubated with the binary topoisomerase–DNA cleaved complex, helps the enzyme to remove itself from the cleaved DNA and close the DNA gap, increasing the religation rate. The compound also induces the religation of the stalled enzyme–CPT (camptothecin)–DNA ternary complex. Analysis of the molecule docked over the binary complex, together with its chemical properties, suggests that the religation enhancement is due to the presence on the compound of two oxygen atoms that act as hydrogen acceptors. This property facilitates the deprotonation of the 5′ DNA end, suggesting that this is the limiting step in the topoisomerase religation mechanism. PMID:23368812

Generalized Hydrodynamic Treatment of the Interplay between Restricted Transport and Catalytic Reactions in Nanoporous Materials

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ackerman, David M.; Wang, Jing; Evans, James W.

2012-05-30

Behavior of catalytic reactions in narrow pores is controlled by a delicate interplay between fluctuations in adsorption-desorption at pore openings, restricted diffusion, and reaction. This behavior is captured by a generalized hydrodynamic formulation of appropriate reaction-diffusion equations (RDE). These RDE incorporate an unconventional description of chemical diffusion in mixed-component quasi-single-file systems based on a refined picture of tracer diffusion for finite-length pores. The RDE elucidate the nonexponential decay of the steady-state reactant concentration into the pore and the non-mean-field scaling of the reactant penetration depth.

Generalized hydrodynamic treatment of the interplay between restricted transport and catalytic reactions in nanoporous materials.

PubMed

Ackerman, David M; Wang, Jing; Evans, James W

2012-06-01

Behavior of catalytic reactions in narrow pores is controlled by a delicate interplay between fluctuations in adsorption-desorption at pore openings, restricted diffusion, and reaction. This behavior is captured by a generalized hydrodynamic formulation of appropriate reaction-diffusion equations (RDE). These RDE incorporate an unconventional description of chemical diffusion in mixed-component quasi-single-file systems based on a refined picture of tracer diffusion for finite-length pores. The RDE elucidate the nonexponential decay of the steady-state reactant concentration into the pore and the non-mean-field scaling of the reactant penetration depth.

Structure of Sn 107 studied through single-neutron knockout reactions

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cerizza, G.; Ayres, A.; Jones, K. L.

2016-02-04

The neutron-deficient nucleus Sn-107 has been studied by using the one-neutron knockout reaction. By measuring the decay gamma rays and momentum distributions of reaction residues, the spins of the ground, 5/2 +, and first-excited, 7/2 +, states of Sn-107 have been assigned by comparisons to eikonal-model reaction calculations. We also observed limits on the inclusive and exclusive cross sections and transitions due to neutron removals from below the N = 50 closed shell have been observed. New excited states up to 5.5 MeV in Sn-107 have been identified.

Low intensity magnetic field influences short-term memory: A study in a group of healthy students.

PubMed

Navarro, Enrique A; Gomez-Perretta, Claudio; Montes, Francisco

2016-01-01

This study analyzes if an external magnetic stimulus (2 kHz and approximately 0.1 μT applied near frontal cortex) influences working memory, perception, binary decision, motor execution, and sustained attention in humans. A magnetic stimulus and a sham stimulus were applied to both sides of the head (frontal cortex close to temporal-parietal area) in young and healthy male test subjects (n = 65) while performing Sternberg's memory scanning task. There was a significant change in reaction time. Times recorded for perception, sustained attention, and motor execution were lower in exposed subjects (P < 0.01). However, time employed in binary decision increased for subjects exposed to magnetic fields. From results, it seems that a low intensity 2 kHz exposure modifies short-term working memory, as well as perception, binary decision, motor execution, and sustained attention. © 2015 Wiley Periodicals, Inc.

Inorganic Halogen Oxidizer Research.

DTIC Science & Technology

1978-01-25

depend on the rate of exchange. Finally, in our experiments we were dealing RI/RD78-125 B-4 -5- with polymeric solid AsF 5 or BF3 phases which on...well be a heterogeneous diffusion controlled reaction and step (5) might be the rate determining step in the above mechanism. It was shown that at...temperatures above -196*C, where a given NF+ salt is still stable in the absence of light, uv irradiation causes a rapid decay RI/RD78-125 B-5 -6- decay of

Porter-Thomas distribution in unstable many-body systems

DOE Office of Scientific and Technical Information (OSTI.GOV)

Volya, Alexander

We use the continuum shell model approach to explore the resonance width distribution in unstable many-body systems. The single-particle nature of a decay, the few-body character of the interaction Hamiltonian, and the collectivity that emerges in nonstationary systems due to the coupling to the continuum of reaction states are discussed. Correlations between the structures of the parent and daughter nuclear systems in the common Fock space are found to result in deviations of decay width statistics from the Porter-Thomas distribution.

Exploring the manifestation and nature of a dineutron in two-neutron emission using a dynamical dineutron model

NASA Astrophysics Data System (ADS)

Grigorenko, L. V.; Vaagen, J. S.; Zhukov, M. V.

2018-03-01

Emission of two neutrons or two protons in reactions and decays is often discussed in terms of "dineutron" or "diproton" emission. The discussion often leans intuitively on something described by Migdal-Watson approximation. In this work we propose a way to formalize situations of dineutron emission. It is demonstrated that properly formally defined dineutron emission may reveal properties which are drastically different from those traditionally expected, and properties which are actually observed in three-body decays.

Extracting information from 0νββ decay and LHC pp-cross sections: Limits on the left-right mixing angle and right-handed boson mass

NASA Astrophysics Data System (ADS)

Civitarese, O.; Suhonen, J.; Zuber, K.

2015-10-01

The existence of massive neutrinos forces the extension of the Standard Model of electroweak interactions, to accommodate them and/or right-handed currents. This is one of the fundamental questions in todays's physics. The consequences of it would reflect upon several decay processes, like the very exotic nuclear double-beta-decay. By the other hand, high-energy proton-proton reactions of the type performed at the LHC accelerator can provide information about the existence of a right-handed generation of the W and Z-bosons. Here we shall address the possibility of performing a joint analysis of the results reported by the ATLAS and CMS collaborations (σ(pp- > 2l + jets)) and the latest measurements of nuclear-double-beta decays reported by the GERDA and EXO collaborations.

Weak decays and double beta decay

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nicholson, H.W.

1983-08-01

Work to measure the ..sigma../sup +/ 0 degree differential cross section in the reaction K/sup -/p ..-->.. ..sigma../sup +/..pi../sup -/ at several incident K/sup -/ momenta between 600 and 800 MeV/c as well as the asymmetries in the decays of polarized ..sigma../sup +/'s into protons and neutral pions and of polarized ..sigma../sup -/'s into neutrons and negative pions in collaboration with experimenters from Yale, Brookhaven, and the University of Pittsburgh (Brookhaven experiment 702) has been completed. Data from this experiment is currently being analyzed at Yale. Work is currently underway to develop and construct an experiment to search for neutrinolessmore » double beta decay in thin foils of Mo/sup 100/ in collaboration with experimenters from Lawrence Berkeley Laboratory. Development work on the solid state silicon detectors should be complete in the next six months and construction should e well underway within the next year.« less

Extracting information from 0νββ decay and LHC pp-cross sections: Limits on the left-right mixing angle and right-handed boson mass

DOE Office of Scientific and Technical Information (OSTI.GOV)

Civitarese, O., E-mail: osvaldo.civitarese@fisica.unlp.edu.ar; Suhonen, J.; Zuber, K.

2015-10-28

The existence of massive neutrinos forces the extension of the Standard Model of electroweak interactions, to accommodate them and/or right-handed currents. This is one of the fundamental questions in todays’s physics. The consequences of it would reflect upon several decay processes, like the very exotic nuclear double-beta-decay. By the other hand, high-energy proton-proton reactions of the type performed at the LHC accelerator can provide information about the existence of a right-handed generation of the W and Z-bosons. Here we shall address the possibility of performing a joint analysis of the results reported by the ATLAS and CMS collaborations (σ(pp− >more » 2l + jets)) and the latest measurements of nuclear-double-beta decays reported by the GERDA and EXO collaborations.« less

Nuclear Data Sheets for A = 251–259 (odd)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Browne, E.; Tuli, J.K.

The evaluators present in this publication spectroscopic data and level schemes from radioactive decay and nuclear reaction studies for all known nuclei with mass numbers A = 251, 253, 255, 257, and 259.

Proton-neutron multiplet states in {sup 112}Sb

DOE Office of Scientific and Technical Information (OSTI.GOV)

Fayez-Hassan, M.; Gulyas, J.; Dombradi, Z.

1997-05-01

Excited states of {sup 112}Sb were investigated through the {sup 112}Sn(p,n{gamma}){sup 112}Sb reaction. {gamma}-ray, {gamma}{gamma}-coincidence, and internal conversion electron spectra were measured with Ge(HP) {gamma} and superconducting magnetic lens plus Si(Li) electron spectrometers at 8.5, 8.9, 9.1, and 9.3 MeV bombarding proton energies. A significantly extended level scheme was constructed. Spins and parities have been assigned to the levels from Hauser-Feshbach analysis of reaction cross sections, internal conversion coefficients, angular distribution of the {gamma} rays, and decay properties of the states. The low lying states were assigned to proton-neutron multiplets on the basis of their decay properties. The energy splittingmore » of these multiplets have been calculated using the parabolic rule. {copyright} {ital 1997} {ital The American Physical Society}« less

Large discrepancies in the excitation function data of the 68Zn(p, x)64Cu reaction: a possible explanation

NASA Astrophysics Data System (ADS)

Steyn, G. F.; Szelecsényi, F.; Kovács, Z.; van der Walt, T. N.; Dolley, S. G.; Vermeulen, C.

2006-05-01

The excitation function of the 68Zn(p, x)64Cu reaction was investigated in an attempt to clarify a serious discrepancy in the recently published data. New measurements based on both a weak γ-line of 1345.8 keV (0.47%) as well as the 511 keV annihilation radiation were performed after radiochemically separating the Cu from the Zn target matrix. In the case of the 511 keV measurements, the method of decay-curve analysis was employed as the annihilation radiation is not specific for a particular radionuclide. The results from the two methods were found to be in excellent agreement. Simulations were also performed to test the method of 511 keV decay-curve analysis for the effects of possible intruder contaminants.

Integral cross section measurement of the U 235 ( n , n ' ) U 235 m reaction in a pulsed reactor

DOE PAGES

Bélier, G.; Bond, E. M.; Vieira, D. J.; ...

2015-04-08

The integral measurement of the neutron inelastic cross section leading to the 26-minute half-life 235mU isomer in a fission-like neutron spectrum is presented. The experiment has been performed at a pulsed reactor, where the internal conversion decay of the isomer was measured using a dedicated electron detector after activation. The sample preparation, efficiency measurement, irradiation, radiochemistry purification, and isomer decay measurement will be presented. We determined the integral cross section for the ²³⁵U(n,n') 235mU reaction to be 1.00±0.13b. This result supports an evaluation performed with TALYS-1.4 code with respect to the isomer excitation as well as the total neutron inelasticmore » scattering cross section.« less

Thermodynamics and kinetics of the sulfation of porous calcium silicate

NASA Technical Reports Server (NTRS)

Miller, R. A.; Kohl, F. J.

1981-01-01

The sulfation of plasma sprayed calcium silicate in flowing SO2/air mixtures at 900 and 1000 C was investigated thermogravimetrically. Reaction products were analyzed using electron microprobe and X-ray diffraction analysis techniques, and results were compared with thermodynamic predictions. The percentage, by volume, of SO2 in air was varied between 0.036 and 10 percent. At 10 percent SO2 the weight gain curve displays a concave downward shoulder early in the sulfation process. An analytical model was developed which treats the initial process as one which decays exponentially with increasing time and the subsequent process as one which decays exponentially with increasing weight gain. At lower SO2 levels the initial rate is controlled by the reactant flow rate. At 1100 C and 0.036 percent SO2 there is no reaction, in agreement with thermodynamic predictions.

Production of bismuth-204 for medical use

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kinsley, M.T.; Lebowitz, E.; Baranosky, J.

1973-11-01

A method is described for producing practical quantities of highpuriti, / sup 204/Bi by, the /sup 206/Pb(p,3n)/sup 204/Bi reaction. A simple elec trolytic separation method with good yield has been developed. The cross section for the above reaction was calculated for 32,MeV protons. Decay data for /supb 204/Bi-/ sup 204m/Pb equilibrium samples are also reported. (auth)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Soker, Noam, E-mail: soker@physics.technion.ac.il

I suggest a spiral-in process in which a stellar companion grazes the envelope of a giant star while both the orbital separation and the giant radius shrink simultaneously, forming a close binary system. The binary system might be viewed as evolving in a constant state of 'just entering a common envelope (CE) phase.' In cases where this process takes place, it can be an alternative to CE evolution where the secondary star is immersed in the giant's envelope. Grazing envelope evolution (GEE) is made possible only if the companion manages to accrete mass at a high rate and launches jetsmore » that remove the outskirts of the giant envelope, hence preventing the formation of a CE. The high accretion rate is made possible by the accretion disk launching jets which efficiently carry the excess angular momentum and energy from the accreted mass. The orbital decay itself is caused by the gravitational interaction of the secondary star with the envelope inward of its orbit, i.e., dynamical friction (gravitational tide). Mass loss through the second Lagrangian point can carry additional angular momentum and envelope mass. The GEE lasts for tens to hundreds of years. The high accretion rate, with peaks lasting from months to years, might lead to a bright object referred to as the intermediate luminosity optical transient (Red Novae; Red Transients). A bipolar nebula and/or equatorial ring are formed around the binary remnant.« less

Direct production of OH radicals upon CH overtone activation of (CH{sub 3}){sub 2}COO Criegee intermediates

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Fang; Beames, Joseph M.; Lester, Marsha I., E-mail: milester@sas.upenn.edu

2014-12-21

Ozonolysis of alkenes, a principle non-photolytic source of atmospheric OH radicals, proceeds through unimolecular decay of energized carbonyl oxide intermediates, known as Criegee intermediates. In this work, cold dimethyl-substituted Criegee intermediates are vibrationally activated in the CH stretch overtone region to drive the 1,4 hydrogen transfer reaction that leads to OH radical products. IR excitation of (CH{sub 3}){sub 2}COO reveals the vibrational states with sufficient oscillator strength, coupling to the reaction coordinate, and energy to surmount the effective barrier (≤ 16.0 kcal mol{sup −1}) to reaction. Insight on the dissociation dynamics is gleaned from homogeneous broadening of the spectral features,more » indicative of rapid intramolecular vibrational energy redistribution and/or reaction, as well as the quantum state distribution of the OH X{sup 2}Π (v = 0) products. The experimental results are compared with complementary electronic structure calculations, which provide the IR absorption spectrum and geometric changes along the intrinsic reaction coordinate. Additional theoretical analysis reveals the vibrational modes and couplings that permit (CH{sub 3}){sub 2}COO to access to the transition state region for reaction. The experimental and theoretical results are compared with an analogous recent study of the IR activation of syn-CH{sub 3}CHOO and its unimolecular decay to OH products [F. Liu, J. M. Beames, A. S. Petit, A. B. McCoy, and M. I. Lester, Science 345, 1596 (2014)].« less

Isovector excitations in 100Nb and their decays by neutron emission studied via the Mo 100 ( t , He 3 + n ) reaction at 115 MeV/u

DOE Office of Scientific and Technical Information (OSTI.GOV)

Miki, K.; Zegers, R. G. T.; Austin, Sam M.

Here, spin–isospin excitations in 100Nb were studied via the charge-exchange reaction at 115 MeV/u with the goal to constrain theoretical models used to describe the isovector spin response of nuclei. The experiment was performed with a secondary beam of tritons, and 3He particles were analyzed in the S800 magnetic spectrometer. Decay by neutron emission from excited states in 100Nb was observed by using plastic and liquid scintillator arrays. Differential cross sections were analyzed and monopole excitations were revealed by using a multipole decomposition analysis. The Gamow–Teller transition strength observed at low excitation energies, which is important for estimating the electron-capturemore » rate in astrophysical scenarios, was strongly fragmented and reduced compared to single-particle and spherical mean-field models. The consideration of deformation in the theoretical estimates was found to be important to better describe the fragmentation and strengths. A strong excitation of the isovector spin giant monopole resonance was observed, and well reproduced by the mean-field models. Its presence makes the extraction of Gamow–Teller strengths at high excitation energies difficult. The branches for statistical and direct decay by neutron emission were identified in the spectra. The upper limit for the branching ratio by direct decay (integrated over all observed excitations) was determined to be 20 ± 6%. Even though the statistical uncertainties in the neutron-coincident data were too large to perform detailed studies of the decay by neutron emission from individual states and resonances, the experiment demonstrates the feasibility of the method.« less

Isovector excitations in 100Nb and their decays by neutron emission studied via the Mo 100 ( t , He 3 + n ) reaction at 115 MeV/u

DOE PAGES

Miki, K.; Zegers, R. G. T.; Austin, Sam M.; ...

2017-04-07

Here, spin–isospin excitations in 100Nb were studied via the charge-exchange reaction at 115 MeV/u with the goal to constrain theoretical models used to describe the isovector spin response of nuclei. The experiment was performed with a secondary beam of tritons, and 3He particles were analyzed in the S800 magnetic spectrometer. Decay by neutron emission from excited states in 100Nb was observed by using plastic and liquid scintillator arrays. Differential cross sections were analyzed and monopole excitations were revealed by using a multipole decomposition analysis. The Gamow–Teller transition strength observed at low excitation energies, which is important for estimating the electron-capturemore » rate in astrophysical scenarios, was strongly fragmented and reduced compared to single-particle and spherical mean-field models. The consideration of deformation in the theoretical estimates was found to be important to better describe the fragmentation and strengths. A strong excitation of the isovector spin giant monopole resonance was observed, and well reproduced by the mean-field models. Its presence makes the extraction of Gamow–Teller strengths at high excitation energies difficult. The branches for statistical and direct decay by neutron emission were identified in the spectra. The upper limit for the branching ratio by direct decay (integrated over all observed excitations) was determined to be 20 ± 6%. Even though the statistical uncertainties in the neutron-coincident data were too large to perform detailed studies of the decay by neutron emission from individual states and resonances, the experiment demonstrates the feasibility of the method.« less

Unveiling hidden properties of young star clusters: differential reddening, star-formation spread, and binary fraction

NASA Astrophysics Data System (ADS)

Bonatto, C.; Lima, E. F.; Bica, E.

2012-04-01

Context. Usually, important parameters of young, low-mass star clusters are very difficult to obtain by means of photometry, especially when differential reddening and/or binaries occur in large amounts. Aims: We present a semi-analytical approach (ASAmin) that, when applied to the Hess diagram of a young star cluster, is able to retrieve the values of mass, age, star-formation spread, distance modulus, foreground and differential reddening, and binary fraction. Methods: The global optimisation method known as adaptive simulated annealing (ASA) is used to minimise the residuals between the observed and simulated Hess diagrams of a star cluster. The simulations are realistic and take the most relevant parameters of young clusters into account. Important features of the simulations are a normal (Gaussian) differential reddening distribution, a time-decreasing star-formation rate, the unresolved binaries, and the smearing effect produced by photometric uncertainties on Hess diagrams. Free parameters are cluster mass, age, distance modulus, star-formation spread, foreground and differential reddening, and binary fraction. Results: Tests with model clusters built with parameters spanning a broad range of values show that ASAmin retrieves the input values with a high precision for cluster mass, distance modulus, and foreground reddening, but they are somewhat lower for the remaining parameters. Given the statistical nature of the simulations, several runs should be performed to obtain significant convergence patterns. Specifically, we find that the retrieved (absolute minimum) parameters converge to mean values with a low dispersion as the Hess residuals decrease. When applied to actual young clusters, the retrieved parameters follow convergence patterns similar to the models. We show how the stochasticity associated with the early phases may affect the results, especially in low-mass clusters. This effect can be minimised by averaging out several twin clusters in the simulated Hess diagrams. Conclusions: Even for low-mass star clusters, ASAmin is sensitive to the values of cluster mass, age, distance modulus, star-formation spread, foreground and differential reddening, and to a lesser degree, binary fraction. Compared with simpler approaches, including binaries, a decaying star-formation rate, and a normally distributed differential reddening appears to yield more constrained parameters, especially the mass, age, and distance from the Sun. A robust determination of cluster parameters may have a positive impact on many fields. For instance, age, mass, and binary fraction are important for establishing the dynamical state of a cluster or for deriving a more precise star-formation rate in the Galaxy.

Dynamics of Db isotopes formed in reactions induced by 238U, 248Cm, and 249Bk across the Coulomb barrier

NASA Astrophysics Data System (ADS)

Kaur, Gurjit; Sandhu, Kirandeep; Kaur, Amandeep; Sharma, Manoj K.

2018-05-01

The dynamical cluster decay model is employed to investigate the decay of *265Db and *267Db nuclei, formed in the 27Al+238U , 18O+249Bk , and 19F+248Cm hot fusion reactions at energies around the Coulomb barrier. First, the fission dynamics of the 27Al+238U reaction is explored by investigating the fragmentation and preformation yield of the reaction. The symmetric mass distribution of the fission fragments is observed for *265Db nucleus, when static β2 i deformations are used within hot optimum orientation approach. However, the mass split gets broaden for the use of β2 i-dynamical hot configuration of the fragments and becomes clearly asymmetric for the cold-static-deformed approach. Within the application of cold orientations of fragments, a new fission channel is observed at mass asymmetry η =0.29 . In addition to 238U-induced reaction, the work is carried out to address the fission and neutron evaporation cross sections of *267Db nucleus formed via 19F+248Cm and 18O+249Bk reactions, besides a comprehensive analysis of fusion and capture processes. Higher fusion cross sections and compound nucleus formation probabilities (PCN) are obtained for the 18O+249Bk reaction, as larger mass asymmetry in the entrance channel leads to reduced Coulomb factor. Finally, the role of sticking (IS) and nonsticking (INS) moments of inertia is analyzed for the 4 n and 5 n channels of *267Db nuclear system.

Synthesis of Binary Transition Metal Nitrides, Carbides and Borides from the Elements in the Laser-Heated Diamond Anvil Cell and Their Structure-Property Relations

PubMed Central

Friedrich, Alexandra; Winkler, Björn; Juarez-Arellano, Erick A.; Bayarjargal, Lkhamsuren

2011-01-01

Transition metal nitrides, carbides and borides have a high potential for industrial applications as they not only have a high melting point but are generally harder and less compressible than the pure metals. Here we summarize recent advances in the synthesis of binary transition metal nitrides, carbides and borides focusing on the reaction of the elements at extreme conditions generated within the laser-heated diamond anvil cell. The current knowledge of their structures and high-pressure properties like high-(p,T) stability, compressibility and hardness is described as obtained from experiments. PMID:28824101

Viscosities of nonelectrolyte liquid mixtures. II. Binary mixtures of n-hexane with alkanoates and bromoalkanoates

NASA Astrophysics Data System (ADS)

Oswal, S. L.; Dave, J. P.

1992-11-01

Viscosity measurements are reported for mixtures of ethyl ethanoate, ethyl propionate, ethyl butyrate, ethyl-2-bromopropionate, ethyl-3-bromopropionate, ethyl-2-bromobutyrate, and ethyl-4-bromobutyrate with n-hexane at 303.15 K. The viscosity data have been correlated with equations of Grunberg and Nissan, of McAllister, and of Auslaender. Furthermore, excess Gibbs energies of activation ΔG * E of viscous flow have been calculated with Eyring's theory of absolute reaction rates and values of ΔG * E for the present binary mixtures have been explained in terms of the dipole-dipole interaction in alkanoates and the intramolecular Br...O interaction in bromoalkanoates.

Catalyst and method for production of methylamines

DOEpatents

Klier, Kamil; Herman, Richard G.; Vedage, Gamini A.

1987-01-01

This invention relates to an improved catalyst and method for the selective production of methylamines. More particularly, it is concerned with the preparation of stable highly active catalysts for producing methylamines by a catalytic reaction of ammonia or substituted amines and binary synthesis gas (CO+H.sub.2).

Test and Evaluation Management Guide, Fifth Edition

DTIC Science & Technology

2005-01-01

determine if a weapon will be useful in combat), chemical weapons testing involves two types of chemical tests—chemical mixing and biotoxicity . Chemical...mixing tests are conducted to obtain in- formation on the binary chemical reaction. Biotoxicity tests are performed to assess the potency of the agent

New Performance Metrics for Quantitative Polymerase Chain Reaction-Based Microbial Source Tracking Methods

EPA Science Inventory

Binary sensitivity and specificity metrics are not adequate to describe the performance of quantitative microbial source tracking methods because the estimates depend on the amount of material tested and limit of detection. We introduce a new framework to compare the performance ...

Reaction rate of the 13C(α,n)16O neutron source using the ANC of the -3 keV resonance measured with the THM

NASA Astrophysics Data System (ADS)

La Cognata, M.; Spitaleri, C.; Trippella, O.; Kiss, G. G.; Rogachev, G. V.; Mukhamedzhanov, A. M.; Avila, M.; Guardo, G. L.; Koshchiy, E.; Kuchera, A.; Lamia, L.; Puglia, S. M. R.; Romano, S.; Santiago, D.; Spartà, R.

2016-01-01

The s-process is responsible of the synthesis of most of the nuclei in the mass range 90 ≤ A ≤ 208. It consists in a series of neutron capture reactions on seed nuclei followed by β-decays, since the neutron accretion rate is slower than the β-decay rate. Such small neutron flux is supplied by the 13C(α,n)16O reaction. It is active inside the helium-burning shell of asymptotic giant branch stars, at temperatures < 108 K, corresponding to an energy interval of 140-230 keV. In this region, the astrophysical S (E)-factor is dominated by the -3 keV sub-threshold resonance due to the 6.356 MeV level in 17O. In this work, we have applied the Trojan Horse Method (THM) to the 13C(6Li,n16O)d quasi-free reaction to extract the 6.356 MeV level resonance parameters, in particular the asymptotic normalization coefficient . A preliminary analysis of a partial data set has lead to , slightly larger than the values in the literature. However, the deduced 13C(α, n)16O reaction rate is in agreement with most results in the literature at ˜ 108 K, with enhanced accuracy thanks to our innovative approach merging together ANC and THM.

Uncertainties in s-process nucleosynthesis in massive stars determined by Monte Carlo variations

NASA Astrophysics Data System (ADS)

Nishimura, N.; Hirschi, R.; Rauscher, T.; St. J. Murphy, A.; Cescutti, G.

2017-08-01

The s-process in massive stars produces the weak component of the s-process (nuclei up to A ˜ 90), in amounts that match solar abundances. For heavier isotopes, such as barium, production through neutron capture is significantly enhanced in very metal-poor stars with fast rotation. However, detailed theoretical predictions for the resulting final s-process abundances have important uncertainties caused both by the underlying uncertainties in the nuclear physics (principally neutron-capture reaction and β-decay rates) as well as by the stellar evolution modelling. In this work, we investigated the impact of nuclear-physics uncertainties relevant to the s-process in massive stars. Using a Monte Carlo based approach, we performed extensive nuclear reaction network calculations that include newly evaluated upper and lower limits for the individual temperature-dependent reaction rates. We found that most of the uncertainty in the final abundances is caused by uncertainties in the neutron-capture rates, while β-decay rate uncertainties affect only a few nuclei near s-process branchings. The s-process in rotating metal-poor stars shows quantitatively different uncertainties and key reactions, although the qualitative characteristics are similar. We confirmed that our results do not significantly change at different metallicities for fast rotating massive stars in the very low metallicity regime. We highlight which of the identified key reactions are realistic candidates for improved measurement by future experiments.

Isobaric yield ratio difference between the 140 A MeV 58Ni + 9Be and 64Ni +9Be reactions studied by the antisymmetric molecular dynamics model

NASA Astrophysics Data System (ADS)

Qiao, C. Y.; Wei, H. L.; Ma, C. W.; Zhang, Y. L.; Wang, S. S.

2015-07-01

Background: The isobaric yield ratio difference (IBD) method is found to be sensitive to the density difference of neutron-rich nucleus induced reaction around the Fermi energy. Purpose: An investigation is performed to study the IBD results in the transport model. Methods: The antisymmetric molecular dynamics (AMD) model plus the sequential decay model gemini are adopted to simulate the 140 A MeV 58 ,64Ni +9Be reactions. A relative small coalescence radius Rc= 2.5 fm is used for the phase space at t = 500 fm/c to form the hot fragment. Two limitations on the impact parameter (b 1 =0 -2 fm and b 2 =0 -9 fm) are used to study the effect of central collisions in IBD. Results: The isobaric yield ratios (IYRs) for the large-A fragments are found to be suppressed in the symmetric reaction. The IBD results for fragments with neutron excess I = 0 and 1 are obtained. A small difference is found in the IBDs with the b 1 and b 2 limitations in the AMD simulated reactions. The IBD with b 1 and b 2 are quite similar in the AMD + GEMINI simulated reactions. Conclusions: The IBDs for the I =0 and 1 chains are mainly determined by the central collisions, which reflects the nuclear density in the core region of the reaction system. The increasing part of the IBD distribution is found due to the difference between the densities in the peripheral collisions of the reactions. The sequential decay process influences the IBD results. The AMD + GEMINI simulation can better reproduce the experimental IBDs than the AMD simulation.

Efficient Green's Function Reaction Dynamics (GFRD) simulations for diffusion-limited, reversible reactions

NASA Astrophysics Data System (ADS)

Bashardanesh, Zahedeh; Lötstedt, Per

2018-03-01

In diffusion controlled reversible bimolecular reactions in three dimensions, a dissociation step is typically followed by multiple, rapid re-association steps slowing down the simulations of such systems. In order to improve the efficiency, we first derive an exact Green's function describing the rate at which an isolated pair of particles undergoing reversible bimolecular reactions and unimolecular decay separates beyond an arbitrarily chosen distance. Then the Green's function is used in an algorithm for particle-based stochastic reaction-diffusion simulations for prediction of the dynamics of biochemical networks. The accuracy and efficiency of the algorithm are evaluated using a reversible reaction and a push-pull chemical network. The computational work is independent of the rates of the re-associations.

Formation and decay of tetrazane derivatives--a Car-Parrinello molecular dynamics study.

PubMed

Nonnenberg, Christel; Frank, Irmgard

2008-08-14

The complications during flight 510 of the Ariane Project were ascribed to problems in the upper stage engine that employs the bipropellant monomethylhydrazine (MMH) and nitrogen tetroxide (NTO). This has led to the question what conditions or reactions possibly cause an uncontrolled behaviour in the combustion process of MMH/NTO. We use first-principles molecular dynamics to investigate the reactions of the hypergolic mixture in different chemical situations. It was possible to observe the ultrafast redox reaction between the reactants on the timescale of an unconstrained simulation. We show that electrostatic attraction is crucial for the understanding of this reaction. Besides a cold reaction preceding the ignition, a reaction path leading to the highly reactive compound dimethyltetrazane could be identified.

A systematic investigation of the (α, 2nγ) reaction on medium-heavy nuclei

NASA Astrophysics Data System (ADS)

Fields, C. A.; De Boer, F. W. N.; Ristinen, R. A.; Smith, P. A.; Sugarbaker, E.

1982-03-01

Exclusive neutron spectra and angular distributions have been measured for 28-35 MeV (α, 2nγ) reactions on various nuclei in the 80 ≦ A ≦ 210 region. Pre-equilibrium processes dominate the 35 MeV (α, 2nγ) reaction mechanism in much of this region. Analysis of systematic variation in the neutron spectrum parameters shows that the reaction mechanism is strongly correlated with the target neutron excess parameter ( N- Z/ A. Analysis of the γ-decay of the entry states shows that well-defined incident angular momentum windows exist for the pre-etjuilibrium (α, 2nγ) reaction. These features are discussed in terms of various models for the reaction mechanism.

X-RAY OUTBURSTS OF ESO 243-49 HLX-1: COMPARISON WITH GALACTIC LOW-MASS X-RAY BINARY TRANSIENTS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yan, Zhen; Zhang, Wenda; Yu, Wenfei

2015-09-20

We studied the outburst properties of the hyper-luminous X-ray source ESO 243-49 HLX-1, using the full set of Swift monitoring observations. We quantified the increase in the waiting time, recurrence time, and e-folding rise timescale along the outburst sequence, and the corresponding decrease in outburst duration, total radiated energy, and e-folding decay timescale, which confirms previous findings. HLX-1 spends less and less time in outburst and more and more time in quiescence, but its peak luminosity remains approximately constant. We compared the HLX-1 outburst properties with those of bright Galactic low-mass X-ray binary transients (LMXBTs). Our spectral analysis strengthens themore » similarity between state transitions in HLX-1 and those in Galactic LMXBTs. We also found that HLX-1 follows the nearly linear correlations between the hard-to-soft state transition luminosity and the peak luminosity, and between the rate of change of X-ray luminosity during the rise phase and the peak luminosity, which indicates that the occurrence of the hard-to-soft state transition of HLX-1 is similar to those of Galactic LMXBTs during outbursts. We found that HLX-1 does not follow the correlations between total radiated energy and peak luminosity, and between total radiated energy and e-folding rise/decay timescales we had previously identified in Galactic LMXBTs. HLX-1 would follow those correlations if the distance were several hundreds of kiloparsecs. However, invoking a much closer distance for HLX-1 is not a viable solution to this problem, as it introduces other, more serious inconsistencies with the observations.« less

KEWPIE2: A cascade code for the study of dynamical decay of excited nuclei

NASA Astrophysics Data System (ADS)

Lü, Hongliang; Marchix, Anthony; Abe, Yasuhisa; Boilley, David

2016-03-01

KEWPIE-a cascade code devoted to investigating the dynamical decay of excited nuclei, specially designed for treating very low probability events related to the synthesis of super-heavy nuclei formed in fusion-evaporation reactions-has been improved and rewritten in C++ programming language to become KEWPIE2. The current version of the code comprises various nuclear models concerning the light-particle emission, fission process and statistical properties of excited nuclei. General features of the code, such as the numerical scheme and the main physical ingredients, are described in detail. Some typical calculations having been performed in the present paper clearly show that theoretical predictions are generally in accordance with experimental data. Furthermore, since the values of some input parameters cannot be determined neither theoretically nor experimentally, a sensibility analysis is presented. To this end, we systematically investigate the effects of using different parameter values and reaction models on the final results. As expected, in the case of heavy nuclei, the fission process has the most crucial role to play in theoretical predictions. This work would be essential for numerical modeling of fusion-evaporation reactions.

C$sup 12$(n,p) B$sup 12$ CROSS SECTION FOR 14.9- TO 17.5-MEV NEUTRONS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kreger, W.E.; Kern, B.D.

1958-09-23

The cross section for the C/sup 12/(n,p)B/sup 12/ reaction has been measured for 14.9- to 17.5-Mev nuetrons. The neutrons were obtained from the T(d,n)He/sup 4/ reaction and their flux density was determined by counting the recoil alpha particles or by counting the neutrons directly with a Li/sup 6/I(Eu) scintillation counter. A cylindrical plastic scintillator 5 inches in diameter and 3 inches in length served as the carbon-containing target and permitted the counting of the B/sup 12/ decay beta rays in nine consecutive 7-msec intervals during the beam-off period or a pulsed neutron beam cycle. The cross section rises from slightlymore » above the reaction threshold of 13.6-Mev to a value of 29.09 plus or minus 4.36 millibarns at 17.5 Mev. The B/sup 12/ beta decay half life has been redetermined as 18.87 plus or minus 0.50 milliseconds. (auth)« less

A novel and facile decay path of Criegee intermediates by intramolecular insertion reactions via roaming transition states

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nguyen, Trong-Nghia; Department of Physical Chemistry, Hanoi University of Science and Technology, Hanoi; Putikam, Raghunath

2015-03-28

We have discovered a new and highly competitive product channel in the unimolecular decay process for small Criegee intermediates, CH{sub 2}OO and anti/syn-CH{sub 3}C(H)OO, occurring by intramolecular insertion reactions via a roaming-like transition state (TS) based on quantum-chemical calculations. Our results show that in the decomposition of CH{sub 2}OO and anti-CH{sub 3}C(H)OO, the predominant paths directly produce cis-HC(O)OH and syn-CH{sub 3}C(O)OH acids with >110 kcal/mol exothermicities via loose roaming-like insertion TSs involving the terminal O atom and the neighboring C–H bonds. For syn-CH{sub 3}C(H)OO, the major decomposition channel occurs by abstraction of a H atom from the CH{sub 3} groupmore » by the terminal O atom producing CH{sub 2}C(H)O–OH. At 298 K, the intramolecular insertion process in CH{sub 2}OO was found to be 600 times faster than the commonly assumed ring-closing reaction.« less

α-cluster versus non-α-cluster decay of the excited compound nucleus Ce124* using the dynamical cluster-decay model

NASA Astrophysics Data System (ADS)

Kaur, Arshdeep; Chopra, Sahila; Gupta, Raj K.

2014-03-01

The dynamical cluster-decay model (DCM), an extended version of the preformed cluster model (PCM) for ground-state (T =0) decays, is applied to study the decay of the proton-rich compound nucleus Ce124* formed in the S32 + Mo92 reaction at an above-barrier beam energy of 150 MeV. Application of the statistical code pace4 to experimental data shows large deviations in all cases of proton clusters' (2p, 3p, and 4p) evaporation residue (ER) and the non-α nucleus Be6 intermediate mass fragment (IMF). Furthermore, the α-nucleus Be8 decay is not observed in this experiment (not even the upper limit is given). Using the DCM, with effects of deformations up to hexadecapole and "compact" orientations included, for the best-fitted cross sections of 2p and 3p ERs and of Li5 and Be6 IMFs, the relative cross section of Be8 is found to be more than that of Be6, possibly due to the α-nucleus structure of Be8. The same is shown to be true for C12 versus C10, i.e., α-nuclei clusters are populated strongly relative to non-α clusters, similar to what was predicted by one of us (R.K.G.) et al. [S. Kumar, D. Bir, and R. K. Gupta, Phys. Rev. C 51, 1762 (1995), 10.1103/PhysRevC.51.1762] for ground-state decays of such nuclei and the decay of Ba116* formed in the Ni58 + Ni58 reaction at various compound nucleus excitation energies [R. K. Gupta et al., J. Phys. G: Nucl. Part. Phys. 32, 345 (2006), 10.1088/0954-3899/32/3/009]. The only parameter of the DCM is the neck-length ΔR, related to the "barrier-lowering" parameter. The compound nucleus formation probability and "barrier-lowering/-modification" effects are analyzed, and the role of varying the deformations of Be6 and/or Be8 nuclei on relative cross sections is studied, since the measured deformations are not available. The ones used here are from relativistic mean-field calculations [β2(6Be )=-0.087 and β2(8Be)=-0.094]. Calculations are also presented for a beam energy of 140 MeV, supporting the above result.

Jetted tidal disruptions of stars as a flag of intermediate mass black holes at high redshifts

NASA Astrophysics Data System (ADS)

Fialkov, Anastasia; Loeb, Abraham

2017-11-01

Tidal disruption events (TDEs) of stars by single or binary supermassive black holes (SMBHs) brighten galactic nuclei and reveal a population of otherwise dormant black holes. Adopting event rates from the literature, we aim to establish general trends in the redshift evolution of the TDE number counts and their observable signals. We pay particular attention to (I) jetted TDEs whose luminosity is boosted by relativistic beaming and (II) TDEs around binary black holes. We show that the brightest (jetted) TDEs are expected to be produced by massive black hole binaries if the occupancy of intermediate mass black holes (IMBHs) in low-mass galaxies is high. The same binary population will also provide gravitational wave sources for the evolved Laser Interferometer Space Antenna. In addition, we find that the shape of the X-ray luminosity function of TDEs strongly depends on the occupancy of IMBHs and could be used to constrain scenarios of SMBH formation. Finally, we make predictions for the expected number of TDEs observed by future X-ray telescopes finding that a 50 times more sensitive instrument than the Burst Alert Telescope (BAT) on board the Swift satellite is expected to trigger ˜10 times more events than BAT, while 6-20 TDEs are expected in each deep field observed by a telescope 50 times more sensitive than the Chandra X-ray Observatory if the occupation fraction of IMBHs is high. Because of their long decay times, high-redshift TDEs can be mistaken for fixed point sources in deep field surveys and targeted observations of the same deep field with year-long intervals could reveal TDEs.

Double-core evolution. 5: Three-dimensional effects in the merger of a red giant with a dwarf companion

NASA Technical Reports Server (NTRS)

Terman, James L.; Taam, Ronald E.; Hernquist, Lars

1994-01-01

The evolution of the common envelope phase of a binary system consisting of a 4.67 solar mass red giant and a 0.94 solar mass dwarf is studied using smoothed particle hydrodynamics. We demonstrate that the three-dimensional effects associated with the gravitational tidal torques lead to a rapid decay of the orbit on timescales approximately less than 1 yr. The relative orbit of the two cores in the common envelope is initally eccentric and tends to circularize as the orbital separation of the two cores decreases. The angular momentum lost from the orbital motion is distributed throughout the common envelope, and the double core does not evolve to a state of co-rotation for the evolutionary time followed. The energy dissipated from the relative orbit and deposited in the common envelope results in the ejection of approximately 13% of the mass of the envelope. The mass is ejected in all directions, but there is a preference for mass ejection in the orbital plane of the binary system. For example, approximately 80% of the ejected mass lies within 30 deg of the binary orbital plane. Because gravitational forces are long range, most of the energy and angular momentum is imparted to a small fraction of the common envelope resulting in an efficiency of the mass ejection process of approximately 15%. The core of the red giant executes significant displacement with respect to the center of mass of the system and contributes nearly equally to the total energy dissipation rate during the latter phases of the evolution. The degree of departure from synchronism of the initial binary system can be an important property of the system which can affect the outcome of the common envelope phase.

Dynamical Aspects of Quasifission Process in Heavy-Ion Reactions

NASA Astrophysics Data System (ADS)

Knyazheva, G. N.; Itkis, I. M.; Kozulin, E. M.

2015-06-01

The study of mass-energy distributions of binary fragments obtained in the reactions of 36S, 48Ca, 58Fe and 64Ni ions with the 232Th, 238U, 244Pu and 248Cm at energies below and above the Coulomb barrier is presented. For all the reactions the main component of the distributions corresponds to asymmetrical mass division typical for asymmetric quasifission process. To describe the quasifission mass distribution the simple method has been proposed. This method is based on the driving potential of the system and time dependent mass drift. This procedure allows to estimate QF time scale from the measured mass distributions. It has been found that the QF time exponentially decreases when the reaction Coulomb factor Z1Z2 increases.

Nuclear Data Sheets for A=40

DOE Office of Scientific and Technical Information (OSTI.GOV)

Chen, Jun

The experimental nuclear structure data and decay data are evaluated for the known nuclides of mass 40 (Mg, Al, Si, P, S, Cl, Ar, K, Ca, Sc, Ti). Detailed evaluated nuclear structure information is presented with the best values recommended for level energies, half-lives, γ-ray energies and intensities, decay properties (energies, intensities and placement of radiations), and other spectroscopic data. The {sup 40}Ca and {sup 40}K nuclides remain as the most extensively studied from many different reactions and decays; no excited states are known in {sup 40}Mg, {sup 40}Al, {sup 40}P and {sup 40}Ti. This work supersedes the earlier fullmore » evaluation of A=40 by J. Cameron and B. Singh (2004Ca38).« less

Nuclear Decay Data for the International Reactor Dosimetry Library for Fission and Fusion (IRDFF): Updated Evaluations of the Half-Lives and Gamma Ray Intensities

NASA Astrophysics Data System (ADS)

Chechev, Valery P.; Kuzmenko, Nikolay K.

2016-02-01

Updated evaluations of the half-lives and prominent gamma ray intensities have been presented for 20 radionuclides - dosimetry reaction residuals. The new values of these decay characteristics recommended for the IRDFF library were obtained using the approaches and methodology adopted by the working group of the Decay Data Evaluation Project (DDEP) cooperation. The experimental data published up to 2014 were taken into account in updated evaluations. The list of radionuclides includes 3H, 18F, 22Na, 24Na, 46Sc, 51Cr, 54Mn, 59Fe, 57Co, 60Co, 57Ni, 64Cu, 88Y, 132Te, 131I, 140Ba, 140La, 141Ce, 182Ta, 198Au.

Search for Invisible Decays of Sub-GeV Dark Photons in Missing-Energy Events at the CERN SPS.

PubMed

Banerjee, D; Burtsev, V; Cooke, D; Crivelli, P; Depero, E; Dermenev, A V; Donskov, S V; Dubinin, F; Dusaev, R R; Emmenegger, S; Fabich, A; Frolov, V N; Gardikiotis, A; Gninenko, S N; Hösgen, M; Kachanov, V A; Karneyeu, A E; Ketzer, B; Kirpichnikov, D V; Kirsanov, M M; Kovalenko, S G; Kramarenko, V A; Kravchuk, L V; Krasnikov, N V; Kuleshov, S V; Lyubovitskij, V E; Lysan, V; Matveev, V A; Mikhailov, Yu V; Myalkovskiy, V V; Peshekhonov, V D; Peshekhonov, D V; Petuhov, O; Polyakov, V A; Radics, B; Rubbia, A; Samoylenko, V D; Tikhomirov, V O; Tlisov, D A; Toropin, A N; Trifonov, A Yu; Vasilishin, B; Vasquez Arenas, G; Ulloa, P; Zhukov, K; Zioutas, K

2017-01-06

We report on a direct search for sub-GeV dark photons (A^{'}), which might be produced in the reaction e^{-}Z→e^{-}ZA^{'} via kinetic mixing with photons by 100 GeV electrons incident on an active target in the NA64 experiment at the CERN SPS. The dark photons would decay invisibly into dark matter particles resulting in events with large missing energy. No evidence for such decays was found with 2.75×10^{9} electrons on target. We set new limits on the γ-A^{'} mixing strength and exclude the invisible A^{'} with a mass ≲100  MeV as an explanation of the muon g_{μ}-2 anomaly.

High-statistics measurement of the η →3 π0 decay at the Mainz Microtron

NASA Astrophysics Data System (ADS)

Prakhov, S.; Abt, S.; Achenbach, P.; Adlarson, P.; Afzal, F.; Aguar-Bartolomé, P.; Ahmed, Z.; Ahrens, J.; Annand, J. R. M.; Arends, H. J.; Bantawa, K.; Bashkanov, M.; Beck, R.; Biroth, M.; Borisov, N. S.; Braghieri, A.; Briscoe, W. J.; Cherepnya, S.; Cividini, F.; Collicott, C.; Costanza, S.; Denig, A.; Dieterle, M.; Downie, E. J.; Drexler, P.; Ferretti Bondy, M. I.; Fil'kov, L. V.; Fix, A.; Gardner, S.; Garni, S.; Glazier, D. I.; Gorodnov, I.; Gradl, W.; Gurevich, G. M.; Hamill, C. B.; Heijkenskjöld, L.; Hornidge, D.; Huber, G. M.; Käser, A.; Kashevarov, V. L.; Kay, S.; Keshelashvili, I.; Kondratiev, R.; Korolija, M.; Krusche, B.; Lazarev, A.; Lisin, V.; Livingston, K.; Lutterer, S.; MacGregor, I. J. D.; Manley, D. M.; Martel, P. P.; McGeorge, J. C.; Middleton, D. G.; Miskimen, R.; Mornacchi, E.; Mushkarenkov, A.; Neganov, A.; Neiser, A.; Oberle, M.; Ostrick, M.; Otte, P. B.; Paudyal, D.; Pedroni, P.; Polonski, A.; Ron, G.; Rostomyan, T.; Sarty, A.; Sfienti, C.; Sokhoyan, V.; Spieker, K.; Steffen, O.; Strakovsky, I. I.; Strandberg, B.; Strub, Th.; Supek, I.; Thiel, A.; Thiel, M.; Thomas, A.; Unverzagt, M.; Usov, Yu. A.; Wagner, S.; Walford, N. K.; Watts, D. P.; Werthmüller, D.; Wettig, J.; Witthauer, L.; Wolfes, M.; Zana, L. A.; A2 Collaboration at MAMI

2018-06-01

The largest, at the moment, statistics of 7 ×106η →3 π0 decays, based on 6.2 ×107η mesons produced in the γ p →η p reaction, has been accumulated by the A2 Collaboration at the Mainz Microtron, MAMI. It allowed a detailed study of the η →3 π0 dynamics beyond its conventional parametrization with just the quadratic slope parameter α and enabled, for the first time, a measurement of the second-order term and a better understanding of the cusp structure in the neutral decay. The present data are also compared to recent theoretical calculations that predict a nonlinear dependence along the quadratic distance from the Dalitz-plot center.

Precision Gamma-Ray Branching Ratios for Long-Lived Radioactive Nuclei

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tonchev, Anton

Many properties of the high-energy-density environments in nuclear weapons tests, advanced laser-fusion experiments, the interior of stars, and other astrophysical bodies must be inferred from the resulting long-lived radioactive nuclei that are produced. These radioactive nuclei are most easily and sensitively identified by studying the characteristic gamma rays emitted during decay. Measuring a number of decays via detection of the characteristic gamma-rays emitted during the gamma-decay (the gamma-ray branching ratio) of the long-lived fission products is one of the most straightforward and reliable ways to determine the number of fissions that occurred in a nuclear weapon test. The fission productsmore » 147Nd, 144Ce, 156Eu, and certain other long-lived isotopes play a crucial role in science-based stockpile stewardship, however, the large uncertainties (about 8%) on the branching ratios measured for these isotopes are currently limiting the usefulness of the existing data [1,2]. We performed highly accurate gamma-ray branching-ratio measurements for a group of high-atomic-number rare earth isotopes to greatly improve the precision and reliability with which the fission yield and reaction products in high-energy-density environments can be determined. We have developed techniques that take advantage of new radioactive-beam facilities, such as DOE's CARIBU located at Argonne National Laboratory, to produce radioactive samples and perform decay spectroscopy measurements. The absolute gamma-ray branching ratios for 147Nd and 144Ce are reduced <2% precision. In addition, high-energy monoenergetic neutron beams from the FN Tandem accelerator in TUNL at Duke University was used to produce 167Tm using the 169Tm(n,3n) reaction. Fourtime improved branching ratio of 167Tm is used now to measure reaction-in-flight (RIF) neutrons from a burning DT capsule at NIF [10]. This represents the first measurement of RIF neutrons in any laboratory fusion system, and the magnitude of the signal has important implications for fundamental plasma science and for weapons physics.« less

Fast analysis of radionuclide decay chain migration

NASA Astrophysics Data System (ADS)

Chen, J. S.; Liang, C. P.; Liu, C. W.; Li, L.

2014-12-01

A novel tool for rapidly predicting the long-term plume behavior of an arbitrary length radionuclide decay chain is presented in this study. This fast tool is achieved based on generalized analytical solutions in compact format derived for a set of two-dimensional advection-dispersion equations coupled with sequential first-order decay reactions in groundwater system. The performance of the developed tool is evaluated by a numerical model using a Laplace transform finite difference scheme. The results of performance evaluation indicate that the developed model is robust and accurate. The developed model is then used to fast understand the transport behavior of a four-member radionuclide decay chain. Results show that the plume extents and concentration levels of any target radionuclide are very sensitive to longitudinal, transverse dispersion, decay rate constant and retardation factor. The developed model are useful tools for rapidly assessing the ecological and environmental impact of the accidental radionuclide releases such as the Fukushima nuclear disaster where multiple radionuclides leaked through the reactor, subsequently contaminating the local groundwater and ocean seawater in the vicinity of the nuclear plant.

Is Deuterium Nuclear Fusion Catalyzed by Antineutrinos?

NASA Astrophysics Data System (ADS)

Shomer, Isaac

2010-02-01

The hypothesis of Fischbach and Jenkins that neutrinos emitted from the sun accelerate radioactive decay is noted. It is thought that neutrinos accelerate beta decay by reacting with neutron-rich nuclides to form a beta particle and a daughter product, with no antineutrino emitted. Conversely, it is proposed that antineutrinos can react with proton-rich nuclides to cause positron decay, with no neutrino emitted. It is also proposed that the nuclear fusion of the hydrogen bomb is triggered not only by the energy of the igniting fission bomb, but by the antineutrinos created by the rapid beta decay of the daughter products in the fission process. The contemplated mechanism for antineutrino initiated fusion is the following: 1. The antineutrinos from the fission daughter products cause positron decay of deuterium by the process outlined above. 2. In a later fusion step, these positrons subsequently react with neutrons in deuterium to create antineutrinos. Electrons are unavailable to annihilate positrons in the plasma of the hydrogen bomb. 3. These antineutrinos thereafter react with more deuterium to form positrons, thereby propagating a chain reaction. )

Decay of 201-203Ra and 200-202Fr

NASA Astrophysics Data System (ADS)

Kalaninová, Z.; Antalic, S.; Andreyev, A. N.; Heßberger, F. P.; Ackermann, D.; Andel, B.; Bianco, L.; Hofmann, S.; Huyse, M.; Kindler, B.; Lommel, B.; Mann, R.; Page, R. D.; Sapple, P. J.; Thomson, J.; Van Duppen, P.; Venhart, M.

2014-05-01

Decay properties of the neutron-deficient nuclides 201-203Ra and 200-202Fr were investigated using α- and γ-decay spectroscopy. The nuclei were produced in fusion-evaporation reactions of 56Fe projectiles with enriched 147Sm and 149Sm targets at the velocity filter SHIP at GSI in Darmstadt (Germany). The α decay from the (3/2-) state in 201Ra was identified with an energy Eα=7842(12) keV and half-life T1/2=8-4+40 ms. Ambiguous decay properties for 202Ra from previous measurements were clarified by remeasuring with significantly improved precision, resulting in values of Eα=7722(7) keV and T1/2=3.8-0.8+1.3 ms. New short-lived isomeric states were identified in 200Fr and 201Fr with half-lives of 0.6-0.2+0.5 μs and 0.7-0.2+0.5 μs, respectively. A tentative spin and parity of 13/2+ were assigned to the latter. One event attributed to β-delayed fission of 200Fr was observed.

Fission of Polyanionic Metal Clusters

NASA Astrophysics Data System (ADS)

König, S.; Jankowski, A.; Marx, G.; Schweikhard, L.; Wolfram, M.

2018-04-01

Size-selected dianionic lead clusters Pbn2 -, n =34 - 56 , are stored in a Penning trap and studied with respect to their decay products upon photoexcitation. Contrary to the decay of other dianionic metal clusters, these lead clusters show a variety of decay channels. The mass spectra of the fragments are compared to the corresponding spectra of the monoanionic precursors. This comparison leads to the conclusion that, in the cluster size region below about n =48 , the fission reaction Pbn2 -→Pbn-10 -+Pb10- is the major decay process. Its disappearance at larger cluster sizes may be an indication of a nonmetal to metal transition. Recently, the pair of Pb10- and Pbn-10 - were observed as pronounced fragments in electron-attachment studies [S. König et al., Int. J. Mass Spectrom. 421, 129 (2017), 10.1016/j.ijms.2017.06.009]. The present findings suggest that this combination is the fingerprint of the decay of doubly charged lead clusters. With this assumption, the dianion clusters have been traced down to Pb212 -, whereas the smallest size for the direct observation was as high as n =28 .

The NUMEN project @ LNS: Status and perspectives

NASA Astrophysics Data System (ADS)

Cappuzzello, F.; Agodi, C.; Acosta, L.; Auerbach, N.; Bellone, J.; Bijker, R.; Bonanno, D.; Bongiovanni, D.; Borello-Lewin, T.; Boztosun, I.; Branchina, V.; Bussa, M. P.; Calabrese, S.; Calabretta, L.; Calanna, A.; Carbone, D.; Cavallaro, M.; Calvo, D.; Lomelí, E. R. Chávez; Coban, A.; Colonna, M.; D'Agostino, G.; Degeronimo, G.; Delaunay, F.; Deshmukh, N.; de Faria, P. N.; Ferraresi, C.; Ferreira, J. L.; Fisichella, M.; Foti, A.; Finocchiaro, P.; Gallo, G.; Garcia, U.; Giraudo, G.; Greco, V.; Hacisalihoglu, A.; Kotila, J.; Iazzi, F.; Introzzi, R.; Lanzalone, G.; Lavagno, A.; Via, F. La; Lay, J. A.; Lenske, H.; Linares, R.; Litrico, G.; Longhitano, F.; Presti, D. Lo; Lubian, J.; Medina, N.; Mendes, D. R.; Muoio, A.; Oliveira, J. R. B.; Pakou, A.; Pandola, L.; Petrascu, H.; Pinna, F.; Reito, S.; Rifuggiato, D.; Rodrigues, M. R. D.; Russo, A. D.; Russo, G.; Santagati, G.; Santopinto, E.; Sgouros, O.; Solakcı, S. O.; Souliotis, G.; Soukeras, V.; Spatafora, A.; Torresi, D.; Tudisco, S.; Vsevolodovna, R. I. M.; Wheadon, R. J.; Yildirin, A.; Zagatto, V.

2017-10-01

The NUMEN project aims at accessing experimentally driven information on Nuclear Matrix Elements (NME) involved in the half-life of the neutrinoless double beta decay (0νββ), by high-accuracy measurements of the cross sections of Heavy Ion (HI) induced Double Charge Exchange (DCE) reactions. Particular attention is given to the (18O,18Ne) and (20Ne,20O) reactions as tools for β+β+ and β-β-decays, respectively. First evidence about the possibility to get quantitative information about NME from experiments is found for both kind of reactions. In the experiments, performed at INFN - Laboratory Nazionali del Sud (LNS) in Catania, the beams are accelerated by the Superconducting Cyclotron (CS) and the reaction products are detected the MAGNEX magnetic spectrometer. The measured cross sections are challengingly low, limiting the present exploration to few selected isotopes of interest in the context of typically low-yield experimental runs. A major upgrade of the LNS facility is foreseen in order to increase the experimental yield of at least two orders of magnitude, thus making feasible a systematic study of all the cases of interest. Frontiers technologies are going to be developed, to this purpose, for the accelerator and the detection systems. In parallel, advanced theoretical models will be developed in order to extract the nuclear structure information from the measured cross sections.

The breakout of the Hot CNO cycle via ^18Ne resonant states

NASA Astrophysics Data System (ADS)

Almaraz-Calderon, S.; Tan, W.; Aprahamian, A.; Bucher, B.; Gorres, J.; Roberts, A.; Villano, A.; Wiescher, M.; Brune, C.; Heinen, Z.; Massey, T.; Ozkan, N.; Guray, R. T.; Mach, H.

2010-11-01

The energy generation rate in the HCNO cycle is limited by the β decay of the waiting point nuclei ^14O and ^15O. However, when the temperatures and densities are high enough (e.g. Novae and X-ray Bursts) it is possible to bypass them by p/α captures resulting in a thermonuclear runaway towards the rp-process. One of the two paths for breakouts from the HCNO cycle is the reaction chain ^14O(α,p)^17F(p,γ)^18Ne(α,p), which proceeds through resonant states on ^18Ne, making their reactions rates very sensitive on the partial and total widths, excitation energies and spins of such resonances. We studied the resonant states in ^18Ne via ^16O(^3He,n) reaction. The neutrons were measured with an array of liquid scintillators using Time-of-Flight and pulse-shape discrimination techniques. The charged particles were detected in coincidence with neutrons by an array of silicon detectors, allowing us to measure α, p, p' and 2p decay branching ratios. Tentative spin assignments were made in comparison with zero range DWBA calculations. This new information will be included in reaction network calculations to evaluate its impact on the nuclear energy generation that occurs in these stellar explosive environments.

Open Charm Yields in d+Au Collisions at sqrt(sNN) = 200 GeV

DOE Office of Scientific and Technical Information (OSTI.GOV)

Adams, J.; Aggarwal, M.M.; Ahammed, Z.

2005-01-07

Mid-rapidity open charm spectra from direct reconstruction of D{sup 0}({bar D}{sup 0}) {yields} K{sup {-+}} {pi}{sup {+-}} in d+Au collisions and indirect electron/positron measurements via charm semileptonic decays in p+p and d+Au collisions at {radical}s{sub NN} = 200 GeV are reported. The D{sup 0}({bar D}{sup 0}) spectrum covers a transverse momentum (p{sub T}) range of 0.1 < p{sub T} < 3 GeV/c whereas the electron spectra cover a range of 1 < p{sub T} < 4 GeV/c. The electron spectra show approximate binary collision scaling between p+p and d+Au collisions. From these two independent analyses, the differential cross section permore » nucleon-nucleon binary interaction at mid-rapidity for open charm production from d+Au collisions at RHIC is d{sigma}{sub c{bar c}}{sup NN}/dy = 0.30 {+-} 0.04 (stat.) {+-} 0.09(syst.) mb. The results are compared to theoretical calculations. Implications for charmonium results in A+A collisions are discussed.« less

Exact statistical results for binary mixing and reaction in variable density turbulence

NASA Astrophysics Data System (ADS)

Ristorcelli, J. R.

2017-02-01

We report a number of rigorous statistical results on binary active scalar mixing in variable density turbulence. The study is motivated by mixing between pure fluids with very different densities and whose density intensity is of order unity. Our primary focus is the derivation of exact mathematical results for mixing in variable density turbulence and we do point out the potential fields of application of the results. A binary one step reaction is invoked to derive a metric to asses the state of mixing. The mean reaction rate in variable density turbulent mixing can be expressed, in closed form, using the first order Favre mean variables and the Reynolds averaged density variance, ⟨ρ2⟩ . We show that the normalized density variance, ⟨ρ2⟩ , reflects the reduction of the reaction due to mixing and is a mix metric. The result is mathematically rigorous. The result is the variable density analog, the normalized mass fraction variance ⟨c2⟩ used in constant density turbulent mixing. As a consequence, we demonstrate that use of the analogous normalized Favre variance of the mass fraction, c″ ⁣2˜ , as a mix metric is not theoretically justified in variable density turbulence. We additionally derive expressions relating various second order moments of the mass fraction, specific volume, and density fields. The central role of the density specific volume covariance ⟨ρ v ⟩ is highlighted; it is a key quantity with considerable dynamical significance linking various second order statistics. For laboratory experiments, we have developed exact relations between the Reynolds scalar variance ⟨c2⟩ its Favre analog c″ ⁣2˜ , and various second moments including ⟨ρ v ⟩ . For moment closure models that evolve ⟨ρ v ⟩ and not ⟨ρ2⟩ , we provide a novel expression for ⟨ρ2⟩ in terms of a rational function of ⟨ρ v ⟩ that avoids recourse to Taylor series methods (which do not converge for large density differences). We have derived analytic results relating several other second and third order moments and see coupling between odd and even order moments demonstrating a natural and inherent skewness in the mixing in variable density turbulence. The analytic results have applications in the areas of isothermal material mixing, isobaric thermal mixing, and simple chemical reaction (in progress variable formulation).

Label-free monitoring of interaction between DNA and oxaliplatin in aqueous solution by terahertz spectroscopy

NASA Astrophysics Data System (ADS)

Wu, Xiaojun; E, Yiwen; Xu, Xinlong; Wang, Li

2012-07-01

We demonstrated the feasibility of applying terahertz time-domain spectroscopy (THz-TDS) to monitor the molecular reactions in aqueous solutions of anticancer drug oxaliplatin with λ-DNA and macrophages DNA. The reaction time dependent refractive index and absorption coefficient were extracted and analyzed. The reaction half-decaying time of about 4.0 h for λ-DNA and 12.9 h for M-DNA was established. The results suggest that the THz-TDS detection could be an effective label-free technique to sense the molecular reaction in aqueous solutions and could be very useful in biology, medicine, and pharmacy industry.

Radiation reaction for spinning bodies in effective field theory. I. Spin-orbit effects

NASA Astrophysics Data System (ADS)

Maia, Natália T.; Galley, Chad R.; Leibovich, Adam K.; Porto, Rafael A.

2017-10-01

We compute the leading post-Newtonian (PN) contributions at linear order in the spin to the radiation-reaction acceleration and spin evolution for binary systems, which enter at fourth PN order. The calculation is carried out, from first principles, using the effective field theory framework for spinning compact objects, in both the Newton-Wigner and covariant spin supplementary conditions. A nontrivial consistency check is performed on our results by showing that the energy loss induced by the resulting radiation-reaction force is equivalent to the total emitted power in the far zone, up to so-called "Schott terms." We also find that, at this order, the radiation reaction has no net effect on the evolution of the spins. The spin-spin contributions to radiation reaction are reported in a companion paper.

Fabrication of hybrid crosslinked network with buffering capabilities and autonomous strengthening characteristics for dental adhesives.

PubMed

Song, Linyong; Ye, Qiang; Ge, Xueping; Misra, Anil; Tamerler, Candan; Spencer, Paulette

2018-02-01

Ingress of bacteria and fluids at the interfacial gaps between the restorative composite biomaterial and the tooth structure contribute to recurrent decay and failure of the composite restoration. The inability of the material to increase the pH at the composite/tooth interface facilitates the outgrowth of bacteria. Neutralizing the microenvironment at the tooth/composite interface offers promise for reducing the damage provoked by cariogenic and aciduric bacteria. We address this problem by designing a dental adhesive composed of hybrid network to provide buffering and autonomous strengthening simultaneously. Two amino functional silanes, 2-hydroxy-3-morpholinopropyl (3-(triethoxysilyl)propyl) carbamate and 2-hydroxy-3-morpholinopropyl (3-(trimethoxysilyl)propyl) carbamate were synthesized and used as co-monomers. Combining free radical initiated polymerization (polymethacrylate-based network) and photoacid-induced sol-gel reaction (polysiloxane) results in the hybrid network formation. Resulting formulations were characterized with regard to real-time photo-polymerization, water sorption, leached species, neutralization, and mechanical properties. Results from real-time FTIR spectroscopic studies indicated that ethoxy was less reactive than methoxy substituent. The neutralization results demonstrated that the methoxy-containing adhesives have acute and delayed buffering capabilities. The mechanical properties of synthetic copolymers tested in dry conditions were improved via condensation reaction of the hydrolyzed organosilanes. The leaching from methoxy containing copolymers was significantly reduced. The sol-gel reaction provided a chronic and persistent reaction in wet condition-performance that offers potential for reducing secondary decay and increasing the functional lifetime of dental adhesives. The interfacial gaps between the restorative composite biomaterial and the tooth structure contributes to recurrent decay and failure of the composite restoration. The inability of the material to increase the pH at the composite/tooth interface facilitates the outgrowth of more cariogenic and aciduric bacteria. This paper reports a novel, synthetic resin that provides buffering capability and autonomous strengthening characteristics. In this work, two amino functional silanes were synthesized and the effect of alkoxy substitutions on the photoacid-induced sol-gel reaction was investigated. We evaluated the neutralization capability (monitoring the pH of lactic acid solution) and the autonomous strengthening property (monitoring the mechanical properties of the hybrid copolymers under wet conditions and quantitatively analyzing the leachable species by HPLC). The novel resin investigated in this study offers the potential benefits of reducing the risk of recurrent decay and prolonging the functional lifetime of dental adhesives. Copyright © 2017 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.

Nuclear Data Sheets for A = 245

DOE Office of Scientific and Technical Information (OSTI.GOV)

Browne, E.; Tuli,J.K.

The evaluators present in this publication spectroscopic data and level schemes from radioactive decay and nuclear reaction studies for all nuclei with mass number A = 245. This evaluation revises the earlier one by Y.A. Akovali (1992Ak05).

Synthesis of superheavy elements at the Dubna gas-filled recoil separator

DOE Office of Scientific and Technical Information (OSTI.GOV)

Voinov, A. A., E-mail: voinov@jinr.ru; Collaboration: JINR

2016-12-15

A survey of experiments at the Dubna gas-filled recoil separator (Laboratory of Nuclear Reactions, JINR, Dubna) aimed at the detection and study of the “island of stability” of superheavy nuclei produced in complete fusion reactions of {sup 48}Ca ions and {sup 238}U–{sup 249}Cf target nuclei is given. The problems of synthesis of superheavy nuclei, methods for their identification, and investigation of their decay properties, including the results of recent experiments at other separators (SHIP, BGS, TASCA) and chemical setups, are discussed. The studied properties of the new nuclei, the isotopes of elements 112–118, as well as the properties of theirmore » decay products, indicate substantial growth of stability of the heaviest nuclei with increasing number of neutrons in the nucleus as the magic number of neutrons N = 184 is approached.« less

Publisher's Note: Branching ratio of the electromagnetic decay of the Σ+(1385) Phys. Rev. D 85, 052004 (2012)

NASA Astrophysics Data System (ADS)

Keller, D.; Hicks, K.; Adhikari, K. P.; Adikaram, D.; Amaryan, M. J.; Anghinolfi, M.; Baghdasaryan, H.; Ball, J.; Battaglieri, M.; Bedlinskiy, I.; Biselli, A. S.; Bookwalter, C.; Boiarinov, S.; Branford, D.; Briscoe, W. J.; Brooks, W. K.; Burkert, V. D.; Carman, D. S.; Celentano, A.; Chandavar, S.; Cole, P. L.; Contalbrigo, M.; Crede, V.; D'Angelo, A.; Daniel, A.; Dashyan, N.; De Vita, R.; De Sanctis, E.; Djalali, C.; Doughty, D.; Dupre, R.; El Alaoui, A.; El Fassi, L.; Elouadrhiri, L.; Eugenio, P.; Fedotov, G.; Gabrielyan, M. Y.; Gevorgyan, N.; Gilfoyle, G. P.; Giovanetti, K. L.; Gohn, W.; Golovatch, E.; Gothe, R. W.; Graham, L.; Griffioen, K. A.; Guidal, M.; Guler, N.; Guo, L.; Hafidi, K.; Hakobyan, H.; Holtrop, M.; Ilieva, Y.; Ireland, D. G.; Ishkhanov, B. S.; Isupov, E. L.; Jo, H. S.; Joo, K.; Khandaker, M.; Khetarpal, P.; Kim, A.; Kim, W.; Klein, F. J.; Kubarovsky, A.; Kubarovsky, V.; Kuleshov, S. V.; Lu, H. Y.; MacGregor, I. J. D.; Mao, Y.; Markov, N.; Mayer, M.; McKinnon, B.; Meyer, C. A.; Mineeva, T.; Mirazita, M.; Mokeev, V.; Moutarde, H.; Munevar, E.; Nadel-Turonski, P.; Nasseripour, R.; Niccolai, S.; Niculescu, G.; Niculescu, I.; Osipenko, M.; Ostrovidov, A. I.; Paolone, M.; Pappalardo, L.; Paremuzyan, R.; Park, K.; Park, S.; Pasyuk, E.; Anefalos Pereira, S.; Pisano, S.; Pogorelko, O.; Pozdniakov, S.; Procureur, S.; Prok, Y.; Protopopescu, D.; Raue, B. A.; Ricco, G.; Rimal, D.; Ripani, M.; Ritchie, B. G.; Rosner, G.; Rossi, P.; Sabatié, F.; Saini, M. S.; Salgado, C.; Schott, D.; Schumacher, R. A.; Seraydaryan, H.; Sharabian, Y. G.; Smith, E. S.; Smith, G. D.; Sober, D. I.; Sokhan, D.; Stepanyan, S. S.; Stepanyan, S.; Stoler, P.; Strauch, S.; Taiuti, M.; Tang, W.; Taylor, C. E.; Tkachenko, S.; Vernarsky, B.; Vineyard, M. F.; Vlassov, A. V.; Voskanyan, H.; Voutier, E.; Watts, D. P.; Wood, M. H.; Zachariou, N.; Zana, L.; Zhao, B.; Zhao, Z. W.

2012-03-01

The CLAS detector was used to obtain the first ever measurement of the electromagnetic decay of the $\\Sigma^{*+}(1385)$ from the reaction $\\gamma p \\to K^0 \\Sigma^{*+}(1385)$. A real photon beam with a maximum energy of 3.8 GeV was incident on a liquid-hydrogen target, resulting in the photoproduction of the kaon and $\\Sigma^*$ hyperon. Kinematic fitting was used to separate the reaction channel from the background processes. The fitting algorithm exploited a new method to kinematically fit neutrons in the CLAS detector, leading to the partial width measurement of $250.0\\pm56.9(stat)^{+34.3}_{-41.2}(sys)$ keV. A U-spin symmetry test using the SU(3) flavor-multiplet representation yields predictions for the $\\Sigma^{*+}(1385)\\to\\Sigma^{+}\\gamma$ and $\\Sigma^{*0}(1385)\\to\\Lambda\\gamma$ partial widths that agree with the experimental measurements.

RAINIER: A simulation tool for distributions of excited nuclear states and cascade fluctuations

NASA Astrophysics Data System (ADS)

Kirsch, L. E.; Bernstein, L. A.

2018-06-01

A new code has been developed named RAINIER that simulates the γ-ray decay of discrete and quasi-continuum nuclear levels for a user-specified range of energy, angular momentum, and parity including a realistic treatment of level spacing and transition width fluctuations. A similar program, DICEBOX, uses the Monte Carlo method to simulate level and width fluctuations but is restricted in its initial level population algorithm. On the other hand, modern reaction codes such as TALYS and EMPIRE populate a wide range of states in the residual nucleus prior to γ-ray decay, but do not go beyond the use of deterministic functions and therefore neglect cascade fluctuations. This combination of capabilities allows RAINIER to be used to determine quasi-continuum properties through comparison with experimental data. Several examples are given that demonstrate how cascade fluctuations influence experimental high-resolution γ-ray spectra from reactions that populate a wide range of initial states.

Gamow-Teller strength observed in the 48Ti(n, p) 48Sc reaction: Implications for the double beta decay of 48Ca

NASA Astrophysics Data System (ADS)

Alford, W. P.; Helmer, R. L.; Abegg, R.; Celler, A.; Frekers, D.; Green, P.; Häusser, O.; Henderson, R.; Hicks, K.; Jackson, K. P.; Jeppesen, R.; Miller, C. A.; Trudel, A.; Vetterli, M.; Yen, S.; Pourang, R.; Watson, J.; Brown, B. A.; Engel, J.

1990-07-01

Cross sections for the 48Ti(n, p) reaction have been measured at angles of 0°, 6°, and 12° at an energy of 200 MeV. The measurements are compared with results of DWIA calculations to obtain estimates of transition strengths for L = 0, 1, and ⩾2 up to an excitation energy of 25 MeV. Gamow-Teller strength ( L = 0) is peaked between 3 and 4 MeV excitation energy, with a significant distribution extending to about 12 MeV. The L = 1 strength is found mainly between 6 and 20 MeV while the cross section for transitions with L ⩾2 increases from 10 MeV to the upper limit of the measurements. The distribution of Gamow-Teller strength is in poor agreement with theoretical distributions used to calculate the lifetime for double beta decay of 48Ca.

Spectroscopic Factors From the Single Neutron Pickup Reaction ^64Zn(d,t)

NASA Astrophysics Data System (ADS)

Leach, Kyle; Garrett, P. E.; Demand, G. A.; Finlay, P.; Green, K. L.; Phillips, A. A.; Sumithrarachchi, C. S.; Svensson, C. E.; Triambak, S.; Ball, G. C.; Faestermann, T.; Krücken, R.; Wirth, H.-F.; Herten-Berger, R.

2008-10-01

A great deal of attention has recently been paid towards high precision superallowed β-decay Ft values. With the availability of extremely high precision (<0.1%) experimental data, the precision on Ft is now limited by the ˜1% theoretical corrections.ootnotetextI.S. Towner and J.C. Hardy, Phys. Rev. C 77, 025501 (2008). This limitation is most evident in heavier superallowed nuclei (e.g. ^62Ga) where the isospin-symmetry-breaking correction calculations become more difficult due to the truncated model space. Experimental data is needed to help constrain input parameters for these calculations, and thus experimental spectroscopic factors for these nuclei are important. Preliminary results from the single-nucleon-transfer reaction ^64Zn(d,t)^63Zn will be presented, and the implications for calculations of isospin-symmetry breaking in the superallowed &+circ; decay of ^62Ga will be discussed.

Radiolabelling of isopeptide N epsilon-(gamma-glutamyl)-L-lysine by conjugation with N-succinimidyl-4-[18F]fluorobenzoate.

PubMed

Wüst, F; Hultsch, C; Bergmann, R; Johannsen, B; Henle, T

2003-07-01

The isopeptide N(epsilon)-(gamma-glutamyl)-L-lysine 4 was labelled with 18F via N-succinimidyl-4-[18F]fluorobenzoate ([18F]SFB). A modified approach for the convenient synthesis of [18F]SFB was used, and [18F]SFB could be obtained in decay-corrected radiochemical yields of 44-53% (n = 20) and radiochemical purity >95% within 40 min after EOB. For labelling N(epsilon)-(gamma-glutamyl)-L-lysine with [18F]SFB the effects of isopeptide concentration, temperature, and pH were studied to determine the optimum reaction conditions. The coupling reaction was shown to be temperature and pH independent while being strongly affected by the isopeptide concentration. Using the optimized labelling conditions, in a typical experiment 1.3GBq of [18F]SFB could be converted into 447MBq (46%, decay-corrected) of [18F]fluorobenzoylated isopeptide within 45 min, including HPLC purification.

Investigation of the Hoyle state in12C with a new hodoscope detector

NASA Astrophysics Data System (ADS)

Dell'Aquila, D.; Lombardo, I.; Vigilante, M.; De Luca, M.; Acosta, L.; Agodi, C.; Cappuzzello, F.; Carbone, D.; Cavallaro, M.; Cherubini, S.; Cvetinovic, A.; D'Agata, G.; Francalanza, L.; Guardo, G. L.; Gulino, M.; Indelicato, I.; La Cognata, M.; Lamia, L.; Ordine, A.; Pizzone, R.; Puglia, S.; Rapisarda, G.; Romano, S.; Santagati, G.; Spartà, R.; Spitaleri, C.; Tumino, A.; Verde, G.

2017-07-01

The {0}2+ state in12C (7.654MeV, the Hoyle state) is important for the understanding of clustering phenomena in nuclei. The pronounced cluster nature of this state allows the triple-α process in stars with a reaction rate regulated by its structure properties. To precisely estimate the direct component in the 3α decay mechanism of the Hoyle state, we developed a new experiment using the14N(d,α)12C reaction at 10.5MeV. An anti-coincidence telescope was used to identify the α ejectiles leading the residual12C in the Hoyle state, while its decays in 3α were studied by means of a new hodoscope of silicon detectors, superOSCAR, placed in kinematical coincidence to fully reconstruct the events. Details of the experiment and preliminary results are discussed in the text.

Branching Ratio of the Electromagnetic Decay of the Σ +(1385)

DOE PAGES

Keller, D.; Hicks, K.; Adhikari, K. P.; ...

2012-03-01

The CLAS detector was used to obtain the first ever measurement of the electromagnetic decay of the Σ* +(1385) from the reaction γp → K 0 Σ* +(1385). A real photon beam with a maximum energy of 3.8 GeV was incident on a liquid-hydrogen target, resulting in the photoproduction of the kaon and Σ* hyperon. Kinematic fitting was used to separate the reaction channel from the background processes. The fitting algorithm exploited a new method to kinematically fit neutrons in the CLAS detector, leading to the partial width measurement of 250.0 ± 56.9(stat) -41.2 +34.3(sys) keV. A U-spin symmetry testmore » using the SU(3) flavor-multiplet representation yields predictions for the Σ* +(1385) → Σ +γ and Σ* 0(1385) → Λγ partial widths that agree with the experimental measurements.« less

Branching Ratio of the Electromagnetic Decay of the Σ +(1385)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Keller, D.; Hicks, K.; Adhikari, K. P.

The CLAS detector was used to obtain the first ever measurement of the electromagnetic decay of the Σ* +(1385) from the reaction γp → K 0 Σ* +(1385). A real photon beam with a maximum energy of 3.8 GeV was incident on a liquid-hydrogen target, resulting in the photoproduction of the kaon and Σ* hyperon. Kinematic fitting was used to separate the reaction channel from the background processes. The fitting algorithm exploited a new method to kinematically fit neutrons in the CLAS detector, leading to the partial width measurement of 250.0 ± 56.9(stat) -41.2 +34.3(sys) keV. A U-spin symmetry testmore » using the SU(3) flavor-multiplet representation yields predictions for the Σ* +(1385) → Σ +γ and Σ* 0(1385) → Λγ partial widths that agree with the experimental measurements.« less

Kinetic model for astaxanthin aggregation in water-methanol mixtures

NASA Astrophysics Data System (ADS)

Giovannetti, Rita; Alibabaei, Leila; Pucciarelli, Filippo

2009-07-01

The aggregation of astaxanthin in hydrated methanol was kinetically studied in the temperature range from 10 °C to 50 °C, at different astaxanthin concentrations and solvent composition. A kinetic model for the formation and transformation of astaxanthin aggregated has been proposed. Spectrophotometric studies showed that monomeric astaxanthin decayed to H-aggregates that after-wards formed J-aggregates when water content was 50% and the temperature lower than 20 °C; at higher temperatures, very stable J-aggregates were formed directly. Monomer formed very stable H-aggregates when the water content was greater than 60%; in these conditions H-aggregates decayed into J-aggregates only when the temperature was at least 50 °C. Through these findings it was possible to establish that the aggregation reactions took place through a two steps consecutive reaction with first order kinetic constants and that the values of these depended on the solvent composition and temperature.

Gamow-Teller Strength Distributions in {sup 48}Sc by the {sup 48}Ca(p,n) and {sup 48}Ti(n,p) Reactions and Two-Neutrino Double-beta Decay Nuclear Matrix Elements

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yako, K.; Sasano, M.; Miki, K.

2009-07-03

The double-differential cross sections for the {sup 48}Ca(p,n) and {sup 48}Ti(n,p) reactions were measured at 300 MeV. A multipole decomposition technique was applied to the spectra to extract the Gamow-Teller (GT) components. The integrated GT strengths up to an excitation energy of 30 MeV in {sup 48}Sc are 15.3+-2.2 and 2.8+-0.3 in the (p,n) and (n,p) spectra, respectively. In the (n,p) spectra additional GT strengths were found above 8 MeV where shell models within the fp shell-model space predict almost no GT strengths, suggesting that the present shell-model description of the nuclear matrix element of the two-neutrino double-beta decay ismore » incomplete.« less

N * → Nη ' decays from photoproduction of η ' -mesons off protons

DOE PAGES

Anisovich, A. V.; Burkert, V.; Collins, P. M.; ...

2017-06-27

We presented a study of the partial-wave content of themore » $$\\gamma p\\to \\eta^\\prime p$$ reaction in the fourth resonance region, which has been prompted by new measurements of polarization observables for that process. Using the Bonn-Gatchina partial-wave formalism, the incorporation of new data indicates that the $N(1895)1/2^-$, $N(1900)3/2^+$, $N(2100)1/2^+$, and $N(2120)3/2^-$ are the most significant contributors to the photoproduction process. Some new results for the branching ratios of the decays of these more prominent resonances to $$N\\eta^\\prime$$ final states are provided; such branches have not been indicated in the most recent edition of the Review of Particle Properties. Based on the analysis performed here, predictions for the helicity asymmetry $E$ for the $$\\gamma p\\to \\eta^\\prime p$$ reaction are presented.« less