Reconstructed plutonium fallout in the GV7 firn core from Northern Victoria Land, East Antarctica

NASA Astrophysics Data System (ADS)

Hwang, H.; Han, Y.; Kang, J.; Lee, K.; Hong, S.; Hur, S. D.; Narcisi, B.; Frezzotti, M.

2017-12-01

Atmospheric nuclear explosions during the period from the 1940s to the 1980s are the major anthropogenic source of plutonium (Pu) in the environment. In this work, we analyzed fg g-1 levels of artificial Pu, released predominantly by atmospheric nuclear weapons tests. We measured 351 samples which collected a 78 m-depth fire core at the site of GV7 (S 70°41'17.1", E 158°51'48.9", 1950 m a.s.l.), Northern Victoria Land, East Antarctica. To determine the Pu concentration in the samples, we used an inductively coupled plasma sector field mass spectrometry coupled with an Apex high-efficiency sample introduction system, which has the advantages of small sample consumption and simple sample preparation. We reconstructed the firn core Pu fallout record for the period after 1954 CE shows a significant fluctuation in agreement with past atmospheric nuclear testing. These data will contribute to ice core research by providing depth-age information.

Atmospheric Impact of Large Methane Emissions and the Gulf Oil Spill

NASA Astrophysics Data System (ADS)

Bhattacharyya, S.; Cameron-Smith, P. J.; Bergmann, D. J.

2010-12-01

A vast quantity of a highly potent greenhouse gas, methane, is locked in the solid phase as methane clathrates in ocean sediments and underneath permafrost regions. Clathrates are ice-like deposits containing a mixture of water and gas (mostly methane) which are stable under high pressure and low temperatures. Current estimates are about 1600 - 2000 GtC present in oceans and about 400GtC in Arctic permafrost (Archer et al. 2009). This is about 4000 times that of current annual emissions. In a warming climate, increase in ocean temperatures could rapidly destabilize the geothermal gradient which in turn could lead to dissociation of the clathrates and release of methane into the ocean and subsequently into the atmosphere as well. This could result in a number of effects including strong greenhouse heating, increased surface ozone, reduced stratospheric ozone, and intensification of the Arctic ozone hole. Many of the effects in the chemistry of the atmosphere are non-linear. In this paper, we present a parametric study of the effect of large scale methane release to the atmosphere. To that end we use the CESM (Community Earth System Model) version 1 with fully active coupled atmosphere-ocean-land model together with super-fast atmospheric chemistry module to simulate the response to increasing CH4 by 2, 3, 10 and 100 times that of the present day. We have also conducted a parametric study of the possible impact of gaseous emissions from the oil spill in the Gulf of Mexico, which is a proxy for future clathrate releases. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

The Navy’s Coupled Atmosphere-Ocean-Wave Prediction System

DTIC Science & Technology

2011-04-15

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Atmospheric Propagation Modeling Indicates Homing Pigeons use Loft-Specific Infrasonic 'Map' Cues

NASA Astrophysics Data System (ADS)

Hagstrum, J. T.; Baker, L. M.; Spritzer, J. M.; McKenna, M. H.

2011-12-01

Pigeons (Columba livia) released at distant sites commonly depart in directions significantly off the actual homeward bearing. Such site-dependent deviations, or biases, for birds from a given loft are generally stable over time, but can also change from hour to hour, day to day, and year to year. At some release sites, birds consistently vanish in random directions and have longer flight times and lower return rates. Release sites characterized by frequent disorientation are not uncommon for pigeon lofts in both Europe and the USA. One such site is the Jersey Hill fire tower in upstate New York located ~120 km W of the Cornell loft in Ithaca. Cornell birds released at Jersey Hill between 1968 and 1987 almost always vanished randomly, although birds from other lofts had little difficulty orienting there. The results for one day, however, stand out: on August 13, 1969, Cornell birds released at Jersey Hill vanished consistently to the NE (r = 0.921; n=7) and returned home after normal flight times. Cornell pigeons released the next day again showed 'normal' behavior for the site and departed randomly. If, in fact, the birds are using acoustic cues to navigate, the long-term acoustic 'dead' zone we propose for Jersey Hill, due to prevailing atmospheric conditions, indicates that the cues are coming from a single, relatively restricted area, most likely surrounding the home loft. We have modeled the transmission of infrasonic waves, presumably coupled to the atmosphere from ocean-generated microseisms (0.14 Hz), between the Cornell loft and a number of release sites using HARPA (Hamiltonian Acoustic Ray-tracing Program for the Atmosphere) and rawinsonde data collected near Albany and Buffalo, NY. The HARPA modeling shows that acoustic signals from the Cornell loft reached Jersey Hill only on a few release days with unusual atmospheric conditions, including August 13, and were launched at angles less than ~2° above horizontal, most likely from steep-sided terrain in the loft vicinity. Such low angles would require sound waves to be diffracted around intervening topography, and likely explains why birds released on August 13 vanished from Jersey Hill at a mean direction to the NE (33°) and not closer to the homeward bearing (85°). Cornell birds released at many sites have departure bearings consistent with such topographic effects. At the Dryden III release site just 13 km E of the Cornell loft, pigeons generally departed to the NW (321°, n=630), ~60° off the homeward bearing (258°). Apparently, infrasonic signals from the home loft area were being diffracted around higher terrain between the loft and release site.

Detailed source term estimation of the atmospheric release for the Fukushima Daiichi Nuclear Power Station accident by coupling simulations of atmospheric dispersion model with improved deposition scheme and oceanic dispersion model

NASA Astrophysics Data System (ADS)

Katata, G.; Chino, M.; Kobayashi, T.; Terada, H.; Ota, M.; Nagai, H.; Kajino, M.; Draxler, R.; Hort, M. C.; Malo, A.; Torii, T.; Sanada, Y.

2014-06-01

Temporal variations in the amount of radionuclides released into the atmosphere during the Fukushima Dai-ichi Nuclear Power Station (FNPS1) accident and their atmospheric and marine dispersion are essential to evaluate the environmental impacts and resultant radiological doses to the public. In this paper, we estimate a detailed time trend of atmospheric releases during the accident by combining environmental monitoring data with atmospheric model simulations from WSPEEDI-II (Worldwide version of System for Prediction of Environmental Emergency Dose Information), and simulations from the oceanic dispersion model SEA-GEARN-FDM, both developed by the authors. A sophisticated deposition scheme, which deals with dry and fogwater depositions, cloud condensation nuclei (CCN) activation and subsequent wet scavenging due to mixed-phase cloud microphysics (in-cloud scavenging) for radioactive iodine gas (I2 and CH3I) and other particles (CsI, Cs, and Te), was incorporated into WSPEEDI-II to improve the surface deposition calculations. The fallout to the ocean surface calculated by WSPEEDI-II was used as input data for the SEA-GEARN-FDM calculations. Reverse and inverse source-term estimation methods based on coupling the simulations from both models was adopted using air dose rates and concentrations, and sea surface concentrations. The results revealed that the major releases of radionuclides due to FNPS1 accident occurred in the following periods during March 2011: the afternoon of 12 March due to the wet venting and hydrogen explosion at Unit 1, the morning of 13 March after the venting event at Unit 3, midnight of 14 March when the SRV (Safely Relief Valve) at Unit 2 was opened three times, the morning and night of 15 March, and the morning of 16 March. According to the simulation results, the highest radioactive contamination areas around FNPS1 were created from 15 to 16 March by complicated interactions among rainfall, plume movements, and the temporal variation of release rates associated with reactor pressure changes in Units 2 and 3. The modified WSPEEDI-II simulation using the new source term reproduced local and regional patterns of cumulative surface deposition of total 131I and 137Cs and air dose rate obtained by airborne surveys. The new source term was also tested using three atmospheric dispersion models (MLDP0, HYSPLIT, and NAME) for regional and global calculations and showed good agreement between calculated and observed air concentration and surface deposition of 137Cs in East Japan. Moreover, HYSPLIT model using the new source term also reproduced the plume arrivals at several countries abroad showing a good correlation with measured air concentration data. A large part of deposition pattern of total 131I and 137Cs in East Japan was explained by in-cloud particulate scavenging. However, for the regional scale contaminated areas, there were large uncertainties due to the overestimation of rainfall amounts and the underestimation of fogwater and drizzle depositions. The computations showed that approximately 27% of 137Cs discharged from FNPS1 deposited to the land in East Japan, mostly in forest areas.

Heinrich events modeled in transient glacial simulations

NASA Astrophysics Data System (ADS)

Ziemen, Florian; Kapsch, Marie; Mikolajewicz, Uwe

2017-04-01

Heinrich events are among the most prominent events of climate variability recorded in proxies across the northern hemisphere. They are the archetype of ice sheet — climate interactions on millennial time scales. Nevertheless, the exact mechanisms that cause Heinrich events are still under debate, and their climatic consequences are far from being fully understood. We address open questions by studying Heinrich events in a coupled ice sheet model (ISM) atmosphere-ocean-vegetation general circulation model (AOVGCM) framework, where this variability occurs as part of the model generated internal variability. The framework consists of a northern hemisphere setup of the modified Parallel Ice Sheet Model (mPISM) coupled to the global AOVGCM ECHAM5/MPIOM/LPJ. The simulations were performed fully coupled and with transient orbital and greenhouse gas forcing. They span from several millennia before the last glacial maximum into the deglaciation. To make these long simulations feasible, the atmosphere is accelerated by a factor of 10 relative to the other model components using a periodical-synchronous coupling technique. To disentangle effects of the Heinrich events and the deglaciation, we focus on the events occurring before the deglaciation. The modeled Heinrich events show a peak ice discharge of about 0.05 Sv and raise the sea level by 2.3 m on average. The resulting surface water freshening reduces the Atlantic meridional overturning circulation and ocean heat release. The reduction in ocean heat release causes a sub-surface warming and decreases the air temperature and precipitation regionally and downstream into Eurasia. The surface elevation decrease of the ice sheet enhances moisture transport onto the ice sheet and thus increases precipitation over the Hudson Bay area, thereby accelerating the recovery after an event.

Exploring the interior of Venus with seismic and infrasonic techniques

NASA Astrophysics Data System (ADS)

Jackson, J. M.; Cutts, J. A.; Pauken, M.; Komjathy, A.; Smrekar, S. E.; Kedar, S.; Mimoun, D.; Garcia, R.; Schubert, G.; Lebonnois, S.; Stevenson, D. J.; Lognonne, P. H.; Zhan, Z.; Ko, J. Y. T.; Tsai, V. C.

2016-12-01

The dense atmosphere of Venus, which efficiently couples seismic energy into the atmosphere as infrasonic waves, enables an alternative to conventional seismology: detection of infrasonic waves in the upper atmosphere using either high altitude balloons or orbiting spacecraft. Infrasonic techniques for probing the interior of Venus can be implemented without exposing sensors to the severe surface environments on Venus. This approach takes advantage of the fact that approximately sixty-times the energy from a seismic event on Venus is coupled into the atmosphere on Venus as would occur for a comparable event on Earth. The direct or epicentral wave propagates vertically above the event, and the indirect wave propagates through the planet as a Rayleigh wave and then couples to an infrasonic wave. Although there is abundant evidence of tectonic activity on Venus, questions remain as to whether the planet is still active and whether energy releases are seismic or aseismic. In recent years, seismologists have developed techniques for probing crustal and interior structure in parts of the Earth where there are very few quakes. We have begun an effort to determine if this is also possible for Venus. Just as seismic energy propagates more efficiently upward across the surface atmosphere interface, equally acoustic energy originating in the atmosphere will propagate downwards more effectively. Measurements from a balloon platform in the atmosphere of Venus could assess the nature and spectral content of such sources, while having the ability to identify and discriminate signatures from volcanic events, storm activity, and meteor impacts. We will discuss our ongoing assessment on the feasibility of a balloon acoustic monitoring system. In particular, we will highlight our results of the flight experiment on Earth that will focus on using barometer instruments on a tethered helium-filled balloon in the vicinity of a known seismic source generated by a seismic hammer. Implications for conducting such measurements on Venus, including seismic and aseismic energy sources and propagation through its atmosphere, will also be discussed.

Diffusive retention of atmospheric gases in chert

NASA Astrophysics Data System (ADS)

Pettitt, E.; Cherniak, D. J.; Watson, E. B.; Schaller, M. F.

2016-12-01

Throughout Earth's history, the volatile contents (N2, CO2, Ar) of both deep and shallow terrestrial reservoirs has been dynamic. Volatiles are important chemical constituents because they play a significant role in regulating Earth's climate, mediating the evolution of complex life, and controlling the properties of minerals and rocks. Estimating levels of atmospheric volatiles in the deep geological past requires interrogation of materials that have acquired and retained a chemical memory from that time. Cherts have the potential to trap atmospheric components during formation and later release those gases for analysis in the laboratory. However, cherts have been underexploited in this regard, partly because their ability to retain a record of volatile components has not been adequately evaluated. Before cherts can be reliably used as indicators of past levels of major atmospheric gases, it is crucial that we understand the diffusive retentiveness of these cryptocrystalline silica phases. As the first step toward quantifying the diffusivity and solubility of carbon dioxide and nitrogen in chert, we have performed 1-atmosphere diffusive-uptake experiments at temperatures up to 450°C. Depth profiles of in-diffusing gases are measured by nuclear reaction analysis (NRA) to help us understand the molecular-scale transport of volatiles and thus the validity of using chert-bound volatiles to record information about Earth history. Data collected to date suggest that at least some cherts are ideal storage containers and can retain volatiles for a geologically long time. In addition to these diffusion experiments, preliminary online-crush fast-scan measurements using a quadrupole mass spectrometer indicate that atmospheric volatiles are released upon crushing various chert samples. By coupling such volatile-release measurements made by mass spectrometry with diffusion experiments, we are uniquely able to address the storage and fidelity of volatiles bound in crustal materials; an important step toward understanding atmospheric evolution over geologic history.

SIRANERISK: Modelling dispersion of steady and unsteady pollutant releases in the urban canopy

NASA Astrophysics Data System (ADS)

Soulhac, L.; Lamaison, G.; Cierco, F.-X.; Ben Salem, N.; Salizzoni, P.; Mejean, P.; Armand, P.; Patryl, L.

2016-09-01

SIRANERISK is an operational model for the simulation of the dispersion of unsteady atmospheric releases of pollutant within and above an urban area. SIRANERISK is built on the same principles as the SIRANE model, and couples a street network model for the pollutant transfers within the urban canopy with a Gaussian puff model for the transfers above it. The performance of the model are here analysed by a detailed comparisons with wind-tunnel experiments. These experiments concern the dispersion of steady and unsteady pollutant releases within and above obstacle arrays with varying geometrical configurations, representing different topologies of idealised urban districts. The overall good agreement between numerical and experimental data demonstrates the reliability of SIRANERISK as an operational tool for the assessment of risk analysis and for the management of crises due to the accidental release of harmful airborne pollutants within a built environment.

Detection of CO2 leaks from carbon capture and storage sites to the atmosphere with combined CO2 and O2 measurements

NASA Astrophysics Data System (ADS)

van Leeuwen, Charlotte; Meijer, Harro A. J.

2015-04-01

One of the main issues in carbon capture and storage (CCS) is the possibility of leakage of CO2 from the storage reservoir to the atmosphere, both from a public health and a climate change combat perspective. Detecting these leaks in the atmosphere is difficult due to the rapid mixing of the emitted CO2 with the surrounding air masses and the high natural variability of the atmospheric CO2 concentration. Instead of measuring only the CO2 concentration of the atmosphere, its isotopes or chemical tracers that are released together with the CO2, our method uses O2 measurements in addition to CO2 measurements to detect a leak from a CCS site. CO2 and O2 are coupled in most processes on earth. In photosynthesis, plants take up CO2 and release O2 at the same time. In respiration and fossil fuel burning, O2 is consumed while CO2 is released. In case of a leak from a CCS site, however, there is no relationship between CO2 and O2. A CO2 leak can therefore be distinguished from other sources of CO2 by looking at the atmospheric CO2-O2 ratio. A natural increase of the CO2 concentration is accompanied by a drop in the O2 concentration, while an increase in the CO2 concentration caused by a leak from a CCS site does not have any effect on the O2 concentration. To demonstrate this leak detection strategy we designed and built a transportable CO2 and O2 measurement system, that is capable of measuring the relatively minute (ppm's variations on a 21% concentration) changes in the O2 concentration. The system comprises of three cases that contain the instrumentation and gas handling equipment, the gas cylinders used as reference and calibration gases and a drying system, respectively. Air is pumped to the system from an air inlet that is placed in a small tower in the field. At the conference, we will demonstrate the success of leak detection with our system by showing measurements of several CO2 release experiments, where CO2 was released at a small distance from the air inlet of our instrument.

A Coupled Soil-Atmosphere Model of H2O2 on Mars

NASA Technical Reports Server (NTRS)

Bullock, Mark A.; Stoker, Carol R.; Mckay, Christopher P.; Zent, Aaron P.

1994-01-01

The Viking Gas Chromatograph Mass Spectrometer failed to detect organic compounds on Mars, and both the Viking Labeled Release and the Viking Gas Exchange experiments indicated a reactive soil surface. These results have led to the widespread belief that there are oxidants in the martian soil. Since H2O2 is produced by photochemical processes in the atmosphere of Mars, and has been shown in the laboratory to reproduce closely the Viking LR results, it is a likely candidate for a martian soil oxidant. Here, we report on the results of a coupled soil/atmosphere transport model for H202 on Mars. Upon diffusing into the soil, its concentration is determined by the extent to which it is adsorbed and by the rate at which it is catalytically destroyed. An analytical model for calculating the distribution of H202 in the martian atmosphere and soil is developed. The concentration of H202 in the soil is shown to go to zero at a finite depth, a consequence of the nonlinear soil diffusion equation. The model is parameterized in terms of an unknown quantity, the lifetime of H202 against heterogeneous catalytic destruction in the soil. Calculated concentrations are compared with a H202 concentration of 30 nmoles/cu cm, inferred from the Viking Labeled Release experiment. A significant result of this model is that for a wide range of H202 lifetimes (up to 105 years), the extinction depth was found to be less than 3 m. The maximum possible concentration in the top 4 cm is calculated to be approx. 240 nmoles/cu cm, achieved with lifetimes of greater than 1000 years. Concentrations higher than 30 nmoles/cu cm require lifetimes of greater than 4.3 terrestrial years. For a wide range of H202 lifetimes, it was found that the atmospheric concentration is only weakly coupled with soil loss processes. Losses to the soil become significant only when lifetimes are less than a few hours. If there are depths below which H202 is not transported, it is plausible that organic compounds, protected from an oxidizing environment, may still exist. They would have been deposited by meteors, or be the organic remains of past life.

Anticipated Improvements to Net Surface Freshwater Fluxes from GPM

NASA Technical Reports Server (NTRS)

Smith, Eric A.

2005-01-01

Evaporation and precipitation over the oceans play very important roles in the global water cycle, upper-ocean heat budget, ocean dynamics, and coupled ocean-atmosphere dynamics. In the conventional representation of the terrestrial water cycle, the assumed role of the oceans is to act as near-infinite reservoirs of water with the main drivers of the water cycle being land- atmosphere interactions in which excess precipitation (P) over evaporation (E) is returned to the oceans as surface runoff and baseflow. Whereas this perspective is valid for short space and time scales -- fundamental principles, available observed estimates, and results from models indicate that the oceans play a far more important role in the large-scale water cycle at seasonal and longer timescales. Approximately 70-80% of the total global evaporation and precipitation occurs over oceans. Moreover, latent heat release into the atmosphere over the oceans is the major heat source driving global atmospheric circulations, with the moisture transported by circulations from oceans to continents being the major source of water precipitating over land. Notably, the major impediment in understanding and modeling the oceans role in the global water cycle is the lack of reliable net surface freshwater flux estimates (E - P fluxes) at the salient spatial and temporal resolutions, i.e., consistent coupled weekly to monthly E - P gridded datasets.

Building-Scale Atmospheric Modeling for Understanding and Anticipating Environmental Risks to Urban Populations

NASA Astrophysics Data System (ADS)

Warner, T. T.; Swerdlin, S. P.; Chen, F.; Hayden, M.

2009-05-01

The innovative use of Computational Fluid-Dynamics (CFD) models to define the building- and street-scale atmospheric environment in urban areas can benefit society in a number of ways. Design criteria used by architectural climatologists, who help plan the livable cities of the future, require information about air movement within street canyons for different seasons and weather regimes. Understanding indoor urban air- quality problems and their mitigation, especially for older buildings, requires data on air movement and associated dynamic pressures near buildings. Learning how heat waves and anthropogenic forcing in cities collectively affect the health of vulnerable residents is a problem in building thermodynamics, human behavior, and neighborhood-scale and street-canyon-scale atmospheric sciences. And, predicting the movement of plumes of hazardous material released in urban industrial or transportation accidents requires detailed information about vertical and horizontal air motions in the street canyons. These challenges are closer to being addressed because of advances in CFD modeling, the coupling of CFD models with models of indoor air motion and air quality, and the coupling of CFD models with mesoscale weather-prediction models. This paper will review some of the new knowledge and technologies that are being developed to meet these atmospheric-environment needs of our growing urban populations.

Ensemble Simulations with Coupled Atmospheric Dynamic and Dispersion Models: Illustrating Uncertainties in Dosage Simulations.

NASA Astrophysics Data System (ADS)

Warner, Thomas T.; Sheu, Rong-Shyang; Bowers, James F.; Sykes, R. Ian; Dodd, Gregory C.; Henn, Douglas S.

2002-05-01

Ensemble simulations made using a coupled atmospheric dynamic model and a probabilistic Lagrangian puff dispersion model were employed in a forensic analysis of the transport and dispersion of a toxic gas that may have been released near Al Muthanna, Iraq, during the Gulf War. The ensemble study had two objectives, the first of which was to determine the sensitivity of the calculated dosage fields to the choices that must be made about the configuration of the atmospheric dynamic model. In this test, various choices were used for model physics representations and for the large-scale analyses that were used to construct the model initial and boundary conditions. The second study objective was to examine the dispersion model's ability to use ensemble inputs to predict dosage probability distributions. Here, the dispersion model was used with the ensemble mean fields from the individual atmospheric dynamic model runs, including the variability in the individual wind fields, to generate dosage probabilities. These are compared with the explicit dosage probabilities derived from the individual runs of the coupled modeling system. The results demonstrate that the specific choices made about the dynamic-model configuration and the large-scale analyses can have a large impact on the simulated dosages. For example, the area near the source that is exposed to a selected dosage threshold varies by up to a factor of 4 among members of the ensemble. The agreement between the explicit and ensemble dosage probabilities is relatively good for both low and high dosage levels. Although only one ensemble was considered in this study, the encouraging results suggest that a probabilistic dispersion model may be of value in quantifying the effects of uncertainties in a dynamic-model ensemble on dispersion model predictions of atmospheric transport and dispersion.

Short-term sea ice forecasts with the RASM-ESRL coupled model: A testbed for improving simulations of ocean-ice-atmosphere interactions in the marginal ice zone

NASA Astrophysics Data System (ADS)

Solomon, A.; Cox, C. J.; Hughes, M.; Intrieri, J. M.; Persson, O. P. G.

2015-12-01

The dramatic decrease of Arctic sea-ice has led to a new Arctic sea-ice paradigm and to increased commercial activity in the Arctic Ocean. NOAA's mission to provide accurate and timely sea-ice forecasts, as explicitly outlined in the National Ocean Policy and the U.S. National Strategy for the Arctic Region, needs significant improvement across a range of time scales to improve safety for human activity. Unfortunately, the sea-ice evolution in the new Arctic involves the interaction of numerous physical processes in the atmosphere, ice, and ocean, some of which are not yet understood. These include atmospheric forcing of sea-ice movement through stress and stress deformation; atmospheric forcing of sea-ice melt and formation through energy fluxes; and ocean forcing of the atmosphere through new regions of seasonal heat release. Many of these interactions involve emerging complex processes that first need to be understood and then incorporated into forecast models in order to realize the goal of useful sea-ice forecasting. The underlying hypothesis for this study is that errors in simulations of "fast" atmospheric processes significantly impact the forecast of seasonal sea-ice retreat in summer and its advance in autumn in the marginal ice zone (MIZ). We therefore focus on short-term (0-20 day) ice-floe movement, the freeze-up and melt-back processes in the MIZ, and the role of storms in modulating stress and heat fluxes. This study uses a coupled ocean-atmosphere-seaice forecast model as a testbed to investigate; whether ocean-sea ice-atmosphere coupling improves forecasts on subseasonal time scales, where systematic biases develop due to inadequate parameterizations (focusing on mixed-phase clouds and surface fluxes), how increased atmospheric resolution of synoptic features improves the forecasts, and how initialization of sea ice area and thickness and snow depth impacts the skill of the forecasts. Simulations are validated with measurements at pan-Arctic land sites, satellite data, and recent ocean field campaigns.

MODTRAN4 radiative transfer modeling for atmospheric correction

NASA Astrophysics Data System (ADS)

Berk, Alexander; Anderson, Gail P.; Bernstein, Lawrence S.; Acharya, Prabhat K.; Dothe, H.; Matthew, Michael W.; Adler-Golden, Steven M.; Chetwynd, James H.; Richtsmeier, Steven C.; Pukall, Brian; Allred, Clark L.; Jeong, Laila S.; Hoke, Michael L.

1999-10-01

MODTRAN4, the latest publicly released version of MODTRAN, provides many new and important options for modeling atmospheric radiation transport. A correlated-k algorithm improves multiple scattering, eliminates Curtis-Godson averaging, and introduces Beer's Law dependencies into the band model. An optimized 15 cm(superscript -1) band model provides over a 10-fold increase in speed over the standard MODTRAN 1 cm(superscript -1) band model with comparable accuracy when higher spectral resolution results are unnecessary. The MODTRAN ground surface has been upgraded to include the effects of Bidirectional Reflectance Distribution Functions (BRDFs) and Adjacency. The BRDFs are entered using standard parameterizations and are coupled into line-of-sight surface radiance calculations.

A deforestation-induced tipping point for the South American monsoon system.

PubMed

Boers, Niklas; Marwan, Norbert; Barbosa, Henrique M J; Kurths, Jürgen

2017-01-25

The Amazon rainforest has been proposed as a tipping element of the earth system, with the possibility of a dieback of the entire ecosystem due to deforestation only of parts of the rainforest. Possible physical mechanisms behind such a transition are still subject to ongoing debates. Here, we use a specifically designed model to analyse the nonlinear couplings between the Amazon rainforest and the atmospheric moisture transport from the Atlantic to the South American continent. These couplings are associated with a westward cascade of precipitation and evapotranspiration across the Amazon. We investigate impacts of deforestation on the South American monsoonal circulation with particular focus on a previously neglected positive feedback related to condensational latent heating over the rainforest, which strongly enhances atmospheric moisture inflow from the Atlantic. Our results indicate the existence of a tipping point. In our model setup, crossing the tipping point causes precipitation reductions of up to 40% in non-deforested parts of the western Amazon and regions further downstream. The responsible mechanism is the breakdown of the aforementioned feedback, which occurs when deforestation reduces transpiration to a point where the available atmospheric moisture does not suffice anymore to release the latent heat needed to maintain the feedback.

A deforestation-induced tipping point for the South American monsoon system

PubMed Central

Boers, Niklas; Marwan, Norbert; Barbosa, Henrique M. J.; Kurths, Jürgen

2017-01-01

The Amazon rainforest has been proposed as a tipping element of the earth system, with the possibility of a dieback of the entire ecosystem due to deforestation only of parts of the rainforest. Possible physical mechanisms behind such a transition are still subject to ongoing debates. Here, we use a specifically designed model to analyse the nonlinear couplings between the Amazon rainforest and the atmospheric moisture transport from the Atlantic to the South American continent. These couplings are associated with a westward cascade of precipitation and evapotranspiration across the Amazon. We investigate impacts of deforestation on the South American monsoonal circulation with particular focus on a previously neglected positive feedback related to condensational latent heating over the rainforest, which strongly enhances atmospheric moisture inflow from the Atlantic. Our results indicate the existence of a tipping point. In our model setup, crossing the tipping point causes precipitation reductions of up to 40% in non-deforested parts of the western Amazon and regions further downstream. The responsible mechanism is the breakdown of the aforementioned feedback, which occurs when deforestation reduces transpiration to a point where the available atmospheric moisture does not suffice anymore to release the latent heat needed to maintain the feedback. PMID:28120928

A deforestation-induced tipping point for the South American monsoon system

NASA Astrophysics Data System (ADS)

Boers, Niklas; Marwan, Norbert; Barbosa, Henrique M. J.; Kurths, Jürgen

2017-01-01

The Amazon rainforest has been proposed as a tipping element of the earth system, with the possibility of a dieback of the entire ecosystem due to deforestation only of parts of the rainforest. Possible physical mechanisms behind such a transition are still subject to ongoing debates. Here, we use a specifically designed model to analyse the nonlinear couplings between the Amazon rainforest and the atmospheric moisture transport from the Atlantic to the South American continent. These couplings are associated with a westward cascade of precipitation and evapotranspiration across the Amazon. We investigate impacts of deforestation on the South American monsoonal circulation with particular focus on a previously neglected positive feedback related to condensational latent heating over the rainforest, which strongly enhances atmospheric moisture inflow from the Atlantic. Our results indicate the existence of a tipping point. In our model setup, crossing the tipping point causes precipitation reductions of up to 40% in non-deforested parts of the western Amazon and regions further downstream. The responsible mechanism is the breakdown of the aforementioned feedback, which occurs when deforestation reduces transpiration to a point where the available atmospheric moisture does not suffice anymore to release the latent heat needed to maintain the feedback.

Coupling a Neural Network with Atmospheric Flow Simulations to Locate and Quantify CH4 Emissions at Well Pads

NASA Astrophysics Data System (ADS)

Travis, B. J.; Sauer, J.; Dubey, M. K.

2017-12-01

Methane (CH4) leaks from oil and gas production fields are a potentially significant source of atmospheric methane. US DOE's ARPA-E office is supporting research to locate methane emissions at 10 m size well pads to within 1 m. A team led by Aeris Technologies, and that includes LANL, Planetary Science Institute and Rice University has developed an autonomous leak detection system (LDS) employing a compact laser absorption methane sensor, a sonic anemometer and multiport sampling. The LDS system analyzes monitoring data using a convolutional neural network (cNN) to locate and quantify CH4 emissions. The cNN was trained using three sources: (1) ultra-high-resolution simulations of methane transport provided by LANL's coupled atmospheric transport model HIGRAD, for numerous controlled methane release scenarios and methane sampling configurations under variable atmospheric conditions, (2) Field tests at the METEC site in Ft. Collins, CO., and (3) Field data from other sites where point-source surface methane releases were monitored downwind. A cNN learning algorithm is well suited to problems in which the training and observed data are noisy, or correspond to complex sensor data as is typical of meteorological and sensor data over a well pad. Recent studies with our cNN emphasize the importance of tracking wind speeds and directions at fine resolution ( 1 second), and accounting for variations in background CH4 levels. A few cases illustrate the importance of sufficiently long monitoring; short monitoring may not provide enough information to determine accurately a leak location or strength, mainly because of short-term unfavorable wind directions and choice of sampling configuration. Length of multiport duty cycle sampling and sample line flush time as well as number and placement of monitoring sensors can significantly impact ability to locate and quantify leaks. Source location error at less than 10% requires about 30 or more training cases.

Remote sensing of methane with OSAS-lidar on the 2ν3 band Q-branch: Experimental proof

NASA Astrophysics Data System (ADS)

Galtier, Sandrine; Anselmo, Christophe; Welschinger, Jean-Yves; Sivignon, J. F.; Cariou, Jean-Pierre; Miffre, Alain; Rairoux, Patrick

2018-06-01

Optical sensors based on absorption spectroscopy play a central role in the detection and monitoring of atmospheric trace gases. We here present for the first time the experimental demonstration of OSAS-Lidar on the remote sensing of CH4 in the atmosphere. This new methodology, the OSAS-Lidar, couples the Optical Similitude Absorption Spectroscopy (OSAS) methodology with a light detection and ranging device. It is based on the differential absorption of spectrally integrated signals following Beer Lambert-Bouguer law, which are range-resolved. Its novelty originates from the use of broadband laser spectroscopy and from the mathematical approach used to retrieve the trace gas concentration. We previously applied the OSAS methodology in laboratory on the 2ν3 methane absorption band, centered at the 1665 nm wavelength and demonstrated that the OSAS-methodology is almost independent from atmospheric temperature and pressure. In this paper, we achieve an OSAS-Lidar device capable of observing large concentrations of CH4 released from a methane source directly into the atmosphere. Comparison with a standard in-situ measurement device shows that the path-integrated concentrations retrieved from OSAS-Lidar methodology exhibit sufficient sensitivity (2 000 ppm m) and observational time resolution (1 s) to remotely sense methane leaks in the atmosphere. The coupling of OSAS-lidar with a wind measurement device opens the way to monitor time-resolved methane flux emissions, which is important in regards to future climate mitigation involving regional reduction of CH4 flux emissions.

Sensitivity of tropical carbon to climate change constrained by carbon dioxide variability.

PubMed

Cox, Peter M; Pearson, David; Booth, Ben B; Friedlingstein, Pierre; Huntingford, Chris; Jones, Chris D; Luke, Catherine M

2013-02-21

The release of carbon from tropical forests may exacerbate future climate change, but the magnitude of the effect in climate models remains uncertain. Coupled climate-carbon-cycle models generally agree that carbon storage on land will increase as a result of the simultaneous enhancement of plant photosynthesis and water use efficiency under higher atmospheric CO(2) concentrations, but will decrease owing to higher soil and plant respiration rates associated with warming temperatures. At present, the balance between these effects varies markedly among coupled climate-carbon-cycle models, leading to a range of 330 gigatonnes in the projected change in the amount of carbon stored on tropical land by 2100. Explanations for this large uncertainty include differences in the predicted change in rainfall in Amazonia and variations in the responses of alternative vegetation models to warming. Here we identify an emergent linear relationship, across an ensemble of models, between the sensitivity of tropical land carbon storage to warming and the sensitivity of the annual growth rate of atmospheric CO(2) to tropical temperature anomalies. Combined with contemporary observations of atmospheric CO(2) concentration and tropical temperature, this relationship provides a tight constraint on the sensitivity of tropical land carbon to climate change. We estimate that over tropical land from latitude 30° north to 30° south, warming alone will release 53 ± 17 gigatonnes of carbon per kelvin. Compared with the unconstrained ensemble of climate-carbon-cycle projections, this indicates a much lower risk of Amazon forest dieback under CO(2)-induced climate change if CO(2) fertilization effects are as large as suggested by current models. Our study, however, also implies greater certainty that carbon will be lost from tropical land if warming arises from reductions in aerosols or increases in other greenhouse gases.

Wave Coupling between the Lower and Middle Thermosphere as Viewed from Quasi-Sun-Synchronous Satellites

NASA Astrophysics Data System (ADS)

Gasperini, Federico

In a society increasingly dependent on space technology, space weather has become a prominent scientific paradigm. In the last decade evidence has shown that terrestrial weather significantly influences space weather. Periodic absorption of solar radiation in local time and longitude by tropospheric water vapor and stratospheric ozone as well as latent heat release in clouds generate a spatially- and temporally-evolving spectrum of global-scale atmospheric waves (i.e., tides, planetary waves and Kelvin waves). A subset of these waves propagates vertically, evolving with height due to wave-mean flow, wave-wave, and wave-plasma interactions, and driving electric fields of tidal origin in the dynamo region. While considerable improvements have been made on the understanding of MLT dynamics, driven in part by the development and deployment of new instruments and techniques, relatively little is known about the coupling of waves in the 120-300 km `thermospheric gap' between satellite remote-sensing and in-situ wave diagnostics. The dissertation herein reveals vertical wave coupling in this height region and quantifies its role in determining thermospheric variability. This objective is accomplished employing quasi-Sun-synchronous satellite measurements (i.e., TIMED, CHAMP, and GOCE) and state-of-the-art numerical modeling simulations (i.e., TIME-GCM/MERRA). Evidence is found for the vertical propagation from the lower to the middle thermosphere of the eastward propagating diurnal tide with zonal wave number 3 (DE3) and the 3-day ultra-fast Kelvin wave (UFKW), two major global-scale atmospheric oscillations of tropospheric origin. These waves are shown to nonlinearly interact and produce secondary waves responsible for significant longitudinal and day-to-day variability. For solar and geomagnetic quiet conditions, atmospheric waves are found to be responsible for up to 60% of the total variability, demonstrating lower atmosphere coupling as a key contributor to thermosphere weather, at least in the absence of major solar-driven variability. Additionally, background atmospheric conditions (i.e., dissipation and zonal mean winds) and found to significantly impact the latitudinal-temporal evolution of upward propagating waves.

Studies in upper and lower atmosphere coupling

NASA Technical Reports Server (NTRS)

Chiu, Y. T.; Rice, C. J.; Sharp, L. R.

1979-01-01

The theoretical and data-analytic work on upper and lower atmosphere coupling performed under a NASA Headquarters contract during the period April 1978 to March 1979 are summarized. As such, this report is primarily devoted to an overview of various studies published and to be published under this contract. Individual study reports are collected as exhibits. Work performed under the subject contract are in the following four areas of upper-lower atmosphere coupling: (1) Magnetosphere-ionosphere electrodynamic coupling in the aurora; (2) Troposphere-thermosphere coupling; (3) Ionosphere-neutral-atmosphere coupling; and (4) Planetary wave dynamics in the middle atmosphere.

A Coupled Surface Nudging Scheme for use in Retrospective ...

EPA Pesticide Factsheets

A surface analysis nudging scheme coupling atmospheric and land surface thermodynamic parameters has been implemented into WRF v3.8 (latest version) for use with retrospective weather and climate simulations, as well as for applications in air quality, hydrology, and ecosystem modeling. This scheme is known as the flux-adjusting surface data assimilation system (FASDAS) developed by Alapaty et al. (2008). This scheme provides continuous adjustments for soil moisture and temperature (via indirect nudging) and for surface air temperature and water vapor mixing ratio (via direct nudging). The simultaneous application of indirect and direct nudging maintains greater consistency between the soil temperature–moisture and the atmospheric surface layer mass-field variables. The new method, FASDAS, consistently improved the accuracy of the model simulations at weather prediction scales for different horizontal grid resolutions, as well as for high resolution regional climate predictions. This new capability has been released in WRF Version 3.8 as option grid_sfdda = 2. This new capability increased the accuracy of atmospheric inputs for use air quality, hydrology, and ecosystem modeling research to improve the accuracy of respective end-point research outcome. IMPACT: A new method, FASDAS, was implemented into the WRF model to consistently improve the accuracy of the model simulations at weather prediction scales for different horizontal grid resolutions, as wel

The case for infrasound as the long-range map cue in avian navigation

USGS Publications Warehouse

Hagstrum, J.T.

2007-01-01

Of the various 'map' and 'compass' components of Kramer's avian navigational model, the long-range map component is the least well understood. In this paper atmospheric infrasounds are proposed as the elusive longrange cues constituting the avian navigational map. Although infrasounds were considered a viable candidate for the avian map in the 1970s, and pigeons in the laboratory were found to detect sounds at surprisingly low frequencies (0.05 Hz), other tests appeared to support either of the currently favored olfactory or magnetic maps. Neither of these hypotheses, however, is able to explain the full set of observations, and the field has been at an impasse for several decades. To begin, brief descriptions of infrasonic waves and their passage through the atmosphere are given, followed by accounts of previously unexplained release results. These examples include 'release-site biases' which are deviations of departing pigeons from the homeward bearing, an annual variation in homing performance observed only in Europe, difficulties orienting over lakes and above temperature inversions, and the mysterious disruption of several pigeon races. All of these irregularities can be consistently explained by the deflection or masking of infrasonic cues by atmospheric conditions or by other infrasonic sources (microbaroms, sonic booms), respectively. A source of continuous geographic infrasound generated by atmosphere-coupled microseisms is also proposed. In conclusion, several suggestions are made toward resolving some of the conflicting experimental data with the pigeons' possible use of infrasonic cues.

New directions: Future approaches to the standardized assessment of airborne pollutants affecting environmental quality

NASA Astrophysics Data System (ADS)

Nehr, Sascha; Franzen-Reuter, Isabelle; Kucejko, Catharina

2017-10-01

Man-made activities have caused unexampled changes of our environment during the last two centuries. Due to emissions of a vast number of pollutants the composition of the Earth's atmosphere is continuously changing, and the consequences for humans and for ecosystems are only partly understood at present. Once released to the atmosphere, the emitted substances undergo physical and chemical degradation. Many of the substances detected in ambient air are toxic or carcinogenic and might cause respiratory and cardiovascular diseases. Furthermore, air pollutants are influencing acidification, eutrophication, global warming, and biodiversity. Therefore soil quality, water quality, air quality, ecosystem exposure to pollutant deposition, biodiversity, and climate change are coupled problems (Schlesinger, 1997; Steffen et al., 2005; Ehlers et al., 2006; Rockström et al., 2009).

On-Line Analysis and Kinetic Behavior of Arsenic Release during Coal Combustion and Pyrolysis.

PubMed

Shen, Fenghua; Liu, Jing; Zhang, Zhen; Dai, Jinxin

2015-11-17

The kinetic behavior of arsenic (As) release during coal combustion and pyrolysis in a fluidized bed was investigated by applying an on-line analysis system of trace elements in flue gas. This system, based on inductively coupled plasma optical emission spectroscopy (ICP-OES), was developed to measure trace elements concentrations in flue gas quantitatively and continuously. Obvious variations of arsenic concentration in flue gas were observed during coal combustion and pyrolysis, indicating strong influences of atmosphere and temperature on arsenic release behavior. Kinetic laws governing the arsenic release during coal combustion and pyrolysis were determined based on the results of instantaneous arsenic concentration in flue gas. A second-order kinetic law was determined for arsenic release during coal combustion, and the arsenic release during coal pyrolysis followed a fourth-order kinetic law. The results showed that the arsenic release rate during coal pyrolysis was faster than that during coal combustion. Thermodynamic calculations were carried out to identify the forms of arsenic in vapor and solid phases during coal combustion and pyrolysis, respectively. Ca3(AsO4)2 and Ca(AsO2)2 are the possible species resulting from As-Ca interaction during coal combustion. Ca(AsO2)2 is the most probable species during coal pyrolysis.

Atmospheric plume progression as a function of time and distance from the release point for radioactive isotopes

DOE Office of Scientific and Technical Information (OSTI.GOV)

Eslinger, Paul W.; Bowyer, Ted W.; Cameron, Ian M.

2015-10-01

The International Monitoring System contains up to 80 stations around the world that have aerosol and xenon monitoring systems designed to detect releases of radioactive materials to the atmosphere from nuclear tests. A rule of thumb description of plume concentration and duration versus time and distance from the release point is useful when designing and deploying new sample collection systems. This paper uses plume development from atmospheric transport modeling to provide a power-law rule describing atmospheric dilution factors as a function of distance from the release point.

Toxicity of atmospheric aerosols on marine phytoplankton

USGS Publications Warehouse

Paytan, A.; Mackey, K.R.M.; Chen, Y.; Lima, I.D.; Doney, S.C.; Mahowald, N.; Labiosa, R.; Post, A.F.

2009-01-01

Atmospheric aerosol deposition is an important source of nutrients and trace metals to the open ocean that can enhance ocean productivity and carbon sequestration and thus influence atmospheric carbon dioxide concentrations and climate. Using aerosol samples from different back trajectories in incubation experiments with natural communities, we demonstrate that the response of phytoplankton growth to aerosol additions depends on specific components in aerosols and differs across phytoplankton species. Aerosol additions enhanced growth by releasing nitrogen and phosphorus, but not all aerosols stimulated growth. Toxic effects were observed with some aerosols, where the toxicity affected picoeukaryotes and Synechococcus but not Prochlorococcus.We suggest that the toxicity could be due to high copper concentrations in these aerosols and support this by laboratory copper toxicity tests preformed with Synechococcus cultures. However, it is possible that other elements present in the aerosols or unknown synergistic effects between these elements could have also contributed to the toxic effect. Anthropogenic emissions are increasing atmospheric copper deposition sharply, and based on coupled atmosphere-ocean calculations, we show that this deposition can potentially alter patterns of marine primary production and community structure in high aerosol, low chlorophyll areas, particularly in the Bay of Bengal and downwind of South and East Asia.

Postglacial response of Arctic Ocean gas hydrates to climatic amelioration

PubMed Central

Serov, Pavel; Mienert, Jürgen; Patton, Henry; Portnov, Alexey; Silyakova, Anna; Panieri, Giuliana; Carroll, Michael L.; Carroll, JoLynn; Andreassen, Karin; Hubbard, Alun

2017-01-01

Seafloor methane release due to the thermal dissociation of gas hydrates is pervasive across the continental margins of the Arctic Ocean. Furthermore, there is increasing awareness that shallow hydrate-related methane seeps have appeared due to enhanced warming of Arctic Ocean bottom water during the last century. Although it has been argued that a gas hydrate gun could trigger abrupt climate change, the processes and rates of subsurface/atmospheric natural gas exchange remain uncertain. Here we investigate the dynamics between gas hydrate stability and environmental changes from the height of the last glaciation through to the present day. Using geophysical observations from offshore Svalbard to constrain a coupled ice sheet/gas hydrate model, we identify distinct phases of subglacial methane sequestration and subsequent release on ice sheet retreat that led to the formation of a suite of seafloor domes. Reconstructing the evolution of this dome field, we find that incursions of warm Atlantic bottom water forced rapid gas hydrate dissociation and enhanced methane emissions during the penultimate Heinrich event, the Bølling and Allerød interstadials, and the Holocene optimum. Our results highlight the complex interplay between the cryosphere, geosphere, and atmosphere over the last 30,000 y that led to extensive changes in subseafloor carbon storage that forced distinct episodes of methane release due to natural climate variability well before recent anthropogenic warming. PMID:28584081

Distributed sensor network for local-area atmospheric modeling

NASA Astrophysics Data System (ADS)

French, Patrick D.; Lovell, John S.; Seaman, Nelson L.

2003-09-01

In the event of a Weapons of Mass Destruction (WMD) chemical or radiological release, quick identification of the nature and source of the release can support efforts to warn, protect and evacuate threatened populations downwind; mitigate the release; provide more accurate plume forecasting; and collect critical transient evidence to help identify the perpetrator(s). Although there are systems available to assist in tracking a WMD release and then predicting where a plume may be traveling, there are no reliable systems available to determine the source location of that release. This would typically require the timely deployment of a remote sensing capability, a grid of expendable air samplers, or a surface sampling plan if the plume has dissipated. Each of these typical solutions has major drawbacks (i.e.: excessive cost, technical feasibility, duration to accomplish, etc...). This paper presents data to support the use of existing rapid-response meteorological modeling coupled with existing transport and diffusion modeling along with a prototype cost-effective situational awareness monitor which would reduce the sensor network requirements while still accomplishing the overall mission of having a 95% probability in converging on a source location within 100 meters.

On the Ni-Ion release rate from surfaces of binary NiTi shape memory alloys

NASA Astrophysics Data System (ADS)

Ševčíková, Jana; Bártková, Denisa; Goldbergová, Monika; Kuběnová, Monika; Čermák, Jiří; Frenzel, Jan; Weiser, Adam; Dlouhý, Antonín

2018-01-01

The study is focused on Ni-ion release rates from NiTi surfaces exposed in the cell culture media and human vascular endothelial cell (HUVEC) culture environments. The NiTi surface layers situated in the depth of 70 μm below a NiTi oxide scale are affected by interactions between the NiTi alloys and the bio-environments. The finding was proved with use of inductively coupled plasma mass spectrometry and electron microscopy experiments. As the exclusive factor controlling the Ni-ion release rates was not only thicknesses of the oxide scale, but also the passivation depth, which was two-fold larger. Our experimental data strongly suggested that some other factors, in addition to the Ni concentration in the oxide scale, admittedly hydrogen soaking deep below the oxide scale, must be taken into account in order to rationalize the concentrations of Ni-ions released into the bio-environments. The suggested role of hydrogen as the surface passivation agent is also in line with the fact that the Ni-ion release rates considerably decrease in NiTi samples that were annealed in controlled hydrogen atmospheres prior to bio-environmental exposures.

Remote sensing observations for monitoring and mathematical simulations of transboundary air pollutants migration from Siberian mass wildfires to Kazakhstan

NASA Astrophysics Data System (ADS)

Kaipov, I. V.

2017-03-01

Anthropogenic and natural factors have increased the power of wildfires in massive Siberian woodlands. As a consequence, the expansion of burned areas and increase in the duration of the forest fire season have led to the release of significant amounts of gases and aerosols. Therefore, it is important to understand the impact of wildland fires on air quality, atmospheric composition, climate and accurately describe the distribution of combustion products in time and space. The most effective research tool is the regional hydrodynamic model of the atmosphere, coupled with the model of pollutants transport and chemical interaction. Taking into account the meteorological parameters and processes of chemical interaction of impurities, complex use of remote sensing techniques for monitoring massive forest fires and mathematical modeling of long-range transport of pollutants in the atmosphere, allow to evaluate spatial and temporal scale of the phenomenon and calculate the quantitative characteristics of pollutants depending on the height and distance of migration.

Evaluation of a Mesoscale Atmospheric Dispersion Modeling System with Observations from the 1980 Great Plains Mesoscale Tracer Field Experiment. Part I: Datasets and Meteorological Simulations.

NASA Astrophysics Data System (ADS)

Moran, Michael D.; Pielke, Roger A.

1996-03-01

The Colorado State University mesoscale atmospheric dispersion (MAD) numerical modeling system, which consists of a prognostic mesoscale meteorological model coupled to a mesoscale Lagrangian particle dispersion model, has been used to simulate the transport and diffusion of a perfluorocarbon tracer-gas cloud for one afternoon surface release during the July 1980 Great Plains mesoscale tracer field experiment. Ground-level concentration (GLC) measurements taken along arcs of samplers 100 and 600 km downwind of the release site at Norman, Oklahoma, up to three days after the tracer release were available for comparison. Quantitative measures of a number of significant dispersion characteristics obtained from analysis of the observed tracer cloud's moving GLC `footprint' have been used to evaluate the modeling system's skill in simulating this MAD case.MAD is more dependent upon the spatial and temporal structure of the transport wind field than is short-range atmospheric dispersion. For the Great Plains mesoscale tracer experiment, the observations suggest that the Great Plains nocturnal low-level jet played an important role in transporting and deforming the tracer cloud. A suite of ten two- and three-dimensional numerical meteorological experiments was devised to investigate the relative contributions of topography, other surface inhomogeneities, atmospheric baroclinicity, synoptic-scale flow evolution, and meteorological model initialization time to the structure and evolution of the low-level mesoscale flow field and thus to MAD. Results from the ten mesoscale meteorological simulations are compared in this part of the paper. The predicted wind fields display significant differences, which give rise in turn to significant differences in predicted low-level transport. The presence of an oscillatory ageostrophic component in the observed synoptic low-level winds for this case is shown to complicate initialization of the meteorological model considerably and is the likely cause of directional errors in the predicted mean tracer transport. A companion paper describes the results from the associated dispersion simulations.

46 CFR 32.63-5 - Barge hull classifications-B/ALL.

Code of Federal Regulations, 2014 CFR

2014-10-01

... the uncontrolled release of the cargo to the waterways and/or atmosphere. (2) Type II barge hull... measures to preclude uncontrolled release to the atmosphere, but whose uncontrolled release to the...

46 CFR 32.63-5 - Barge hull classifications-B/ALL.

Code of Federal Regulations, 2013 CFR

2013-10-01

... the uncontrolled release of the cargo to the waterways and/or atmosphere. (2) Type II barge hull... measures to preclude uncontrolled release to the atmosphere, but whose uncontrolled release to the...

An innovative coupling between column leaching and oxygen consumption tests to assess behavior of contaminated marine dredged sediments.

PubMed

Couvidat, Julien; Benzaazoua, Mostafa; Chatain, Vincent; Zhang, Fan; Bouzahzah, Hassan

2015-07-01

Contaminated dredged sediments are often considered hazardous wastes, so they have to be adequately managed to avoid leaching of pollutants. The mobility of inorganic contaminants is a major concern. Metal sulfides (mainly framboïdal pyrite, copper, and zinc sulfides) have been investigated in this study as an important reactive metal-bearing phase sensitive to atmospheric oxygen action. An oxygen consumption test (OC-Test) has been adapted to assess the reactivity of dredged sediments when exposed to atmospheric oxygen. An experimental column set-up has been developed allowing the coupling between leaching and oxygen consumption test to investigate the reactivity of the sediment. This reactivity, which consisted of sulfide oxidation, was found to occur for saturation degree between 60 and 90 % and until the 20th testing week, through significant sulfates releases. These latter were assumed to come from sulfide oxidation in the first step of the test, then probably from gypsum dissolution. Confrontation results of OC-Test and leachate quality shows that Cu was well correlated to sulfates releases, which in turn, leads to Ca and Mg dissolution (buffer effect). Cu, and mostly Zn, was associated to organic matter, phyllosilicates, and other minerals through organo-clay complexes. This research confirmed that the OC-Test, originally developed for mine tailings, could be a useful tool in the dredged sediment field which can allow for intrinsic characterization of reactivity of a material suspected to readily reacting with oxygen and for better understanding of geochemical processes that affect pollutants behavior, conversion, and transfer in the environment.

Estimating trace gas and aerosol emissions over South America: Relationship between fire radiative energy released and aerosol optical depth observations

NASA Astrophysics Data System (ADS)

Pereira, Gabriel; Freitas, Saulo R.; Moraes, Elisabete Caria; Ferreira, Nelson Jesus; Shimabukuro, Yosio Edemir; Rao, Vadlamudi Brahmananda; Longo, Karla M.

2009-12-01

Contemporary human activities such as tropical deforestation, land clearing for agriculture, pest control and grassland management lead to biomass burning, which in turn leads to land-cover changes. However, biomass burning emissions are not correctly measured and the methods to assess these emissions form a part of current research area. The traditional methods for estimating aerosols and trace gases released into the atmosphere generally use emission factors associated with fuel loading and moisture characteristics and other parameters that are hard to estimate in near real-time applications. In this paper, fire radiative power (FRP) products were extracted from Moderate Resolution Imaging Spectroradiometer (MODIS) and from the Geostationary Operational Environmental Satellites (GOES) fire products and new South America generic biomes FRE-based smoke aerosol emission coefficients were derived and applied in 2002 South America fire season. The inventory estimated by MODIS and GOES FRP measurements were included in Coupled Aerosol-Tracer Transport model coupled to the Brazilian developments on the Regional Atmospheric Modeling System (CATT-BRAMS) and evaluated with ground truth collected in Large Scale Biosphere-Atmosphere Smoke, Aerosols, Clouds, rainfall, and Climate (SMOCC) and Radiation, Cloud, and Climate Interactions (RaCCI). Although the linear regression showed that GOES FRP overestimates MODIS FRP observations, the use of a common external parameter such as MODIS aerosol optical depth product could minimize the difference between sensors. The relationship between the PM 2.5μm (Particulate Matter with diameter less than 2.5 μm) and CO (Carbon Monoxide) model shows a good agreement with SMOCC/RaCCI data in the general pattern of temporal evolution. The results showed high correlations, with values between 0.80 and 0.95 (significant at 0.5 level by student t test), for the CATT-BRAMS simulations with PM 2.5μm and CO.

Computed and observed turbulent heat fluxes during an extreme Bora event in the Adriatic using atmosphere-ocean coupling

NASA Astrophysics Data System (ADS)

Ličer, Matjaž; Smerkol, Peter; Fettich, Anja; Ravdas, Michalis; Papapostolou, Alexandros; Mantziafou, Anneta; Strajnar, Benedikt; Cedilnik, Jure; Jeromel, Maja; Jerman, Jure; Petan, Sašo; Benetazzo, Alvise; Carniel, Sandro; Malačič, Vlado; Sofianos, Sarantis

2016-04-01

We have studied the performances of (a) a two-way coupled atmosphere-ocean modeling system and (b) one-way coupled ocean model (forced by the atmosphere model), as compared to the available in situ measurements during and after a strong Adriatic Bora wind event in February 2012, which led to extreme air-sea interactions. The simulations span the period between January and March 2012. The models used were ALADIN (4.4 km resolution) on the atmosphere side and Adriatic setup of POM (1°/30 × 1°/30 angular resolution) on the ocean side. The atmosphere-ocean coupling was implemented using the OASIS3-MCT model coupling toolkit. Two-way coupling ocean feedback to the atmosphere is limited to sea surface temperature. We have compared modeled atmosphere-ocean fluxes (computed using modified Louis scheme) and sea temperatures from both setups to platform and CTD measurements of fluxes (computed using COARE scheme) and temperatures from three observational platforms (Vida, Paloma, Acqua Alta) in the Northern Adriatic. We show that turbulent fluxes from both setups differ up to 20% during the Bora but not significantly before and after the event. The impact of the coupling on the ocean is significant while the impact on the atmosphere is less pronounced. When compared to observations, two way coupling ocean temperatures exhibit a four times lower RMSE than those from one-way coupled system. Two-way coupling improves sensible heat fluxes at all stations but does not improve latent heat loss.

Ocean-Atmosphere Coupling Processes Affecting Predictability in the Climate System

NASA Astrophysics Data System (ADS)

Miller, A. J.; Subramanian, A. C.; Seo, H.; Eliashiv, J. D.

2017-12-01

Predictions of the ocean and atmosphere are often sensitive to coupling at the air-sea interface in ways that depend on the temporal and spatial scales of the target fields. We will discuss several aspects of these types of coupled interactions including oceanic and atmospheric forecast applications. For oceanic mesoscale eddies, the coupling can influence the energetics of the oceanic flow itself. For Madden-Julian Oscillation onset, the coupling timestep should resolve the diurnal cycle to properly raise time-mean SST and latent heat flux prior to deep convection. For Atmospheric River events, the evolving SST field can alter the trajectory and intensity of precipitation anomalies along the California coast. Improvements in predictions will also rely on identifying and alleviating sources of biases in the climate states of the coupled system. Surprisingly, forecast skill can also be improved by enhancing stochastic variability in the atmospheric component of coupled models as found in a multiscale ensemble modeling approach.

The Aliso Canyon Natural Gas Leak : Large Eddy Simulations for Modeling Atmospheric Dynamics and Interpretation of Observations.

NASA Astrophysics Data System (ADS)

Prasad, K.; Thorpe, A. K.; Duren, R. M.; Thompson, D. R.; Whetstone, J. R.

2016-12-01

The National Institute of Standards and Technology (NIST) has supported the development and demonstration of a measurement capability to accurately locate greenhouse gas sources and measure their flux to the atmosphere over urban domains. However, uncertainties in transport models which form the basis of all top-down approaches can significantly affect our capability to attribute sources and predict their flux to the atmosphere. Reducing uncertainties between bottom-up and top-down models will require high resolution transport models as well as validation and verification of dispersion models over an urban domain. Tracer experiments involving the release of Perfluorocarbon Tracers (PFTs) at known flow rates offer the best approach for validating dispersion / transport models. However, tracer experiments are limited by cost, ability to make continuous measurements, and environmental concerns. Natural tracer experiments, such as the leak from the Aliso Canyon underground storage facility offers a unique opportunity to improve and validate high resolution transport models, test leak hypothesis, and to estimate the amount of methane released.High spatial resolution (10 m) Large Eddy Simulations (LES) coupled with WRF atmospheric transport models were performed to simulate the dynamics of the Aliso Canyon methane plume and to quantify the source. High resolution forward simulation results were combined with aircraft and tower based in-situ measurements as well as data from NASA airborne imaging spectrometers. Comparison of simulation results with measurement data demonstrate the capability of the LES models to accurately model transport and dispersion of methane plumes over urban domains.

Wildland Fire Forecasting: Predicting Wildfire Behavior, Growth, and Feedbacks on Weather

NASA Astrophysics Data System (ADS)

Coen, J. L.

2005-12-01

Recent developments in wildland fire research models have represented more complex of fire behavior. The cost has been to increase the computational requirements. When operational constraints are included, such as the need to produce such forecasts faster than real time, the challenge becomes a balance of how much complexity (with corresponding gains in realism) and accuracy can be achieved in producing the quantities of interest while meeting the specified operational constraints. Current field tools are calculator or Palm-Pilot based algorithms such as BEHAVE and BEHAVE Plus that produce timely estimates of instantaneous fire spread rates, flame length, and fire intensity at a point using readily estimated inputs of fuel model, terrain slope, and atmospheric wind speed at a point. At the cost of requiring a PC and slower calculation, FARSITE represents two-dimensional fire spread and adds capabilities including a parameterized representation of crown fire ignition, This work describes how a coupled atmosphere-fire model previously used as a research tool has been adapted for production of real-time forecasts of fire growth and its interactions with weather over a domain focusing on Colorado during summer 2004. The coupled atmosphere-wildland fire-environment (CAWFE) model composed of a 3-dimensional atmospheric prediction model that has been two-way coupled with an empirical fire spread model. The models are connected in that atmospheric conditions (and fuel conditions influenced by the atmosphere) affect the rate and direction of fire propagation, which releases sensible and latent heat (i.e. thermal and water vapor fluxes) to the atmosphere that in turn alter the winds and atmospheric structure around the fire. Thus, it can represent time and spatially-varying weather and the fire feedbacks on the atmospheric which are at the heart of sudden changes in fire behavior and examples of extreme fire behavior such as blow ups, which are now not predictable with current tools. Thus, although this work shows that is it possible to perform more detailed simulations in real time, fire behavior forecasting remains a challenging problem. This is due to challenges in weather prediction, particularly at fine spatial and temporal scales considered "nowcasting" (0-6 hrs), uncertainties in fire behavior even with known meteorological conditions, limitations in quantitative datasets on fuel properties such as fuel loading, and verification. This work describes efforts to advance these capabilities with input from remote sensing data on fuel characteristics and dynamic steering and object-based verification with remotely sensed fire perimeters.

Infiltration and Evaporation of Diesel and Gasoline Droplets Spilled onto Concrete Pavement

NASA Astrophysics Data System (ADS)

Hilpert, M.; Adria-Mora, B.

2015-12-01

Pollution at gas stations due to small spills that occur during refueling of customer vehicles has received little attention. We have performed laboratory experiments in order to assess the processes of evaporation and infiltration of fuel spilled onto concrete samples. Changes in mass of both spilled diesel and gasoline droplets as a function of time have been analyzed. The infiltrated mass is affected by variations in humidity, among other parameters, which influence the amount of water condensed onto the concrete. Therefore, we used a humidity data logger and statistical tools to predict the evolution of the real mass of infiltrated fuel. The infiltrated mass roughly decreases exponentially, but the difference in behavior between both fuel types is important. The percentage of evaporated mass is much larger for gasoline, while infiltration is more significant for diesel. Also, the percentage of infiltrated liquid depends on the initial droplet mass. We also developed a multiphysics model, which couples pore-scale infiltration to turbulent atmospheric transport, to explain the experimental data. In conclusion, a substantial amount of fuel could both seep into the ground to contaminate groundwater and be released to the atmosphere. More studies are needed to quantify the public health implications of the released pollutants.

Development of capability for microtopography-resolving simulations of hydrologic processes in permafrost affected regions

NASA Astrophysics Data System (ADS)

Painter, S.; Moulton, J. D.; Berndt, M.; Coon, E.; Garimella, R.; Lewis, K. C.; Manzini, G.; Mishra, P.; Travis, B. J.; Wilson, C. J.

2012-12-01

The frozen soils of the Arctic and subarctic regions contain vast amounts of stored organic carbon. This carbon is vulnerable to release to the atmosphere as temperatures warm and permafrost degrades. Understanding the response of the subsurface and surface hydrologic system to degrading permafrost is key to understanding the rate, timing, and chemical form of potential carbon releases to the atmosphere. Simulating the hydrologic system in degrading permafrost regions is challenging because of the potential for topographic evolution and associated drainage network reorganization as permafrost thaws and massive ground ice melts. The critical process models required for simulating hydrology include subsurface thermal hydrology of freezing/thawing soils, thermal processes within ice wedges, mechanical deformation processes, overland flow, and surface energy balances including snow dynamics. A new simulation tool, the Arctic Terrestrial Simulator (ATS), is being developed to simulate these coupled processes. The computational infrastructure must accommodate fully unstructured grids that track evolving topography, allow accurate solutions on distorted grids, provide robust and efficient solutions on highly parallel computer architectures, and enable flexibility in the strategies for coupling among the various processes. The ATS is based on Amanzi (Moulton et al. 2012), an object-oriented multi-process simulator written in C++ that provides much of the necessary computational infrastructure. Status and plans for the ATS including major hydrologic process models and validation strategies will be presented. Highly parallel simulations of overland flow using high-resolution digital elevation maps of polygonal patterned ground landscapes demonstrate the feasibility of the approach. Simulations coupling three-phase subsurface thermal hydrology with a simple thaw-induced subsidence model illustrate the strong feedbacks among the processes. D. Moulton, M. Berndt, M. Day, J. Meza, et al., High-Level Design of Amanzi, the Multi-Process High Performance Computing Simulator, Technical Report ASCEM-HPC-2011-03-1, DOE Environmental Management, 2012.

Modulated Hawking radiation and a nonviolent channel for information release

NASA Astrophysics Data System (ADS)

Giddings, Steven B.

2014-11-01

Unitarization of black hole evaporation requires that quantum information escapes a black hole; an important question is to identify the mechanism or channel by which it does so. Accurate counting of black hole states via the Bekenstein-Hawking entropy would indicate this information should be encoded in radiation with average energy flux matching Hawking's. Information can be encoded with no change in net flux via fine-grained modulation of the Hawking radiation. In an approximate effective field theory description, couplings to the stress tensor of the black hole atmosphere that depend on the internal state of the black hole are a promising alternative for inducing such modulation. These can be picturesquely thought of as due to state-dependent metric fluctuations in the vicinity of the horizon. Such couplings offer the prospect of emitting information without extra energy flux, and can be shown to do so at linear order in the couplings, with motivation given for possible extension of this result to higher orders. The potential advantages of such couplings to the stress tensor thus extend beyond their universality, which is helpful in addressing constraints from black hole mining.

Modeling short-term concentration fluctuations of semi-volatile pollutants in the soil-plant-atmosphere system.

PubMed

Bao, Zhongwen; Haberer, Christina M; Maier, Uli; Beckingham, Barbara; Amos, Richard T; Grathwohl, Peter

2016-11-01

Temperature changes can drive cycling of semi-volatile pollutants between different environmental compartments (e.g. atmosphere, soil, plants). To evaluate the impact of daily temperature changes on atmospheric concentration fluctuations we employed a physically based model coupling soil, plants and the atmosphere, which accounts for heat transport, effective gas diffusion, sorption and biodegradation in the soil as well as eddy diffusion and photochemical oxidation in the atmospheric boundary layer of varying heights. The model results suggest that temperature-driven re-volatilization and uptake in soils cannot fully explain significant diurnal concentration fluctuations of atmospheric pollutants as for example observed for polychlorinated biphenyls (PCBs). This holds even for relatively low water contents (high gas diffusivity) and high sorption capacity of the topsoil (high organic carbon content and high pollutant concentration in the topsoil). Observed concentration fluctuations, however, can be easily matched if a rapidly-exchanging environmental compartment, such as a plant layer, is introduced. At elevated temperatures, plants release organic pollutants, which are rapidly distributed in the atmosphere by eddy diffusion. For photosensitive compounds, e.g. some polycyclic aromatic hydrocarbons (PAHs), decreasing atmospheric concentrations would be expected during daytime for the bare soil scenario. This decline is buffered by a plant layer, which acts as a ground-level reservoir. The modeling results emphasize the importance of a rapidly-exchanging compartment above ground to explain short-term atmospheric concentration fluctuations. Copyright © 2016 Elsevier B.V. All rights reserved.

The Met Office Coupled Atmosphere/Land/Ocean/Sea-Ice Data Assimilation System

NASA Astrophysics Data System (ADS)

Lea, Daniel; Mirouze, Isabelle; King, Robert; Martin, Matthew; Hines, Adrian

2015-04-01

The Met Office has developed a weakly-coupled data assimilation (DA) system using the global coupled model HadGEM3 (Hadley Centre Global Environment Model, version 3). At present the analysis from separate ocean and atmosphere DA systems are combined to produced coupled forecasts. The aim of coupled DA is to produce a more consistent analysis for coupled forecasts which may lead to less initialisation shock and improved forecast performance. The HadGEM3 coupled model combines the atmospheric model UM (Unified Model) at 60 km horizontal resolution on 85 vertical levels, the ocean model NEMO (Nucleus for European Modelling of the Ocean) at 25 km (at the equator) horizontal resolution on 75 vertical levels, and the sea-ice model CICE at the same resolution as NEMO. The atmosphere and the ocean/sea-ice fields are coupled every 1-hour using the OASIS coupler. The coupled model is corrected using two separate 6-hour window data assimilation systems: a 4D-Var for the atmosphere with associated soil moisture content nudging and snow analysis schemes on the one hand, and a 3D-Var FGAT for the ocean and sea-ice on the other hand. The background information in the DA systems comes from a previous 6-hour forecast of the coupled model. To isolate the impact of the coupled DA, 13-month experiments have been carried out, including 1) a full atmosphere/land/ocean/sea-ice coupled DA run, 2) an atmosphere-only run forced by OSTIA SSTs and sea-ice with atmosphere and land DA, and 3) an ocean-only run forced by atmospheric fields from run 2 with ocean and sea-ice DA. In addition, 5-day and 10-day forecast runs, have been produced from initial conditions generated by either run 1 or a combination of runs 2 and 3. The different results have been compared to each other and, whenever possible, to other references such as the Met Office atmosphere and ocean operational analyses or the OSTIA SST data. The performance of the coupled DA is similar to the existing separate ocean and atmosphere DA systems. This is despite the fact that the assimilation error covariances have not yet been tuned for coupled DA. In addition, the coupled model also exhibits some biases which do not affect the uncoupled models. An example is precipitation and run off errors affecting the ocean salinity. This of course impacts the performance of the ocean data assimilation. This does, however, highlight a particular benefit of data assimilation in that it can help to identify short term model biases by using, for example, the differences between the observations and model background (innovations) and the mean increments. Coupled DA has the distinct advantage that this gives direct information about the coupled model short term biases. By identifying the biases and developing solutions this will improve the short range coupled forecasts, and may also improve the coupled model on climate timescales.

Simulation of seasonal anomalies of atmospheric circulation using coupled atmosphere-ocean model

NASA Astrophysics Data System (ADS)

Tolstykh, M. A.; Diansky, N. A.; Gusev, A. V.; Kiktev, D. B.

2014-03-01

A coupled atmosphere-ocean model intended for the simulation of coupled circulation at time scales up to a season is developed. The semi-Lagrangian atmospheric general circulation model of the Hydrometeorological Centre of Russia, SLAV, is coupled with the sigma model of ocean general circulation developed at the Institute of Numerical Mathematics, Russian Academy of Sciences (INM RAS), INMOM. Using this coupled model, numerical experiments on ensemble modeling of the atmosphere and ocean circulation for up to 4 months are carried out using real initial data for all seasons of an annual cycle in 1989-2010. Results of these experiments are compared to the results of the SLAV model with the simple evolution of the sea surface temperature. A comparative analysis of seasonally averaged anomalies of atmospheric circulation shows prospects in applying the coupled model for forecasts. It is shown with the example of the El Niño phenomenon of 1997-1998 that the coupled model forecasts the seasonally averaged anomalies for the period of the nonstationary El Niño phase significantly better.

Intraseasonal and interannual oscillations in coupled ocean-atmosphere models

NASA Technical Reports Server (NTRS)

Hirst, Anthony C.; Lau, K.-M.

1990-01-01

An investigation is presented of coupled ocean-atmosphere models' behavior in an environment where atmospheric wave speeds are substantially reduced from dry atmospheric values by such processes as condensation-moisture convergence. Modes are calculated for zonally periodic, unbounded ocean-atmosphere systems, emphasizing the importance of an inclusion of prognostic atmosphere equations in simple coupled ocean-atmosphere models with a view to simulations of intraseasonal variability and its possible interaction with interannual variability. The dynamics of low and high frequency modes are compared; both classes are sensitive to the degree to which surface wind anomalies are able to affect the evaporation rate.

Coupling between geochemical reactions and multicomponent gas and solute transport in unsaturated media: A reactive transport modeling study

USGS Publications Warehouse

Molins, S.; Mayer, K.U.

2007-01-01

The two‐way coupling that exists between biogeochemical reactions and vadose zone transport processes, in particular gas phase transport, determines the composition of soil gas. To explore these feedback processes quantitatively, multicomponent gas diffusion and advection are implemented into an existing reactive transport model that includes a full suite of geochemical reactions. Multicomponent gas diffusion is described on the basis of the dusty gas model, which accounts for all relevant gas diffusion mechanisms. The simulation of gas attenuation in partially saturated landfill soil covers, methane production, and oxidation in aquifers contaminated by organic compounds (e.g., an oil spill site) and pyrite oxidation in mine tailings demonstrate that both diffusive and advective gas transport can be affected by geochemical reactions. Methane oxidation in landfill covers reduces the existing upward pressure gradient, thereby decreasing the contribution of advective methane emissions to the atmosphere and enhancing the net flux of atmospheric oxygen into the soil column. At an oil spill site, methane oxidation causes a reversal in the direction of gas advection, which results in advective transport toward the zone of oxidation both from the ground surface and the deeper zone of methane production. Both diffusion and advection contribute to supply atmospheric oxygen into the subsurface, and methane emissions to the atmosphere are averted. During pyrite oxidation in mine tailings, pressure reduction in the reaction zone drives advective gas flow into the sediment column, enhancing the oxidation process. In carbonate‐rich mine tailings, calcite dissolution releases carbon dioxide, which partly offsets the pressure reduction caused by O2 consumption.

Modeling the Entry of Micrometeoroids into the Atmospheres of Earth-like Planets

NASA Technical Reports Server (NTRS)

Pevyhouse, A. R.; Kress, M. E.

2011-01-01

The temperature profiles of micrometeors entering the atmospheres of Earth-like planets are calculated to determine the altitude at which exogenous organic compounds may be released. Previous experiments have shown that flash-heated micrometeorite analogs release organic compounds at temperatures from roughly 500 to 1000 K [1]. The altitude of release is of great importance because it determines the fate of the compound. Organic compounds that are released deeper in the atmosphere are more likely to rapidly mix to lower altitudes where they can accumulate to higher abundances or form more complex molecules and/or aerosols. Variables that are explored here are particle size, entry angle, atmospheric density profiles, spectral type of the parent star, and planet mass. The problem reduces to these questions: (1) How much atmosphere does the particle pass through by the time it is heated to 500 K? (2) Is the atmosphere above sufficient to attenuate stellar UV such that the mixing timescale is shorter than the photochemical timescale for a particular compound? We present preliminary results that the effect of the planetary and particle parameters have on the altitude of organic release.

The impact of SciDAC on US climate change research and the IPCCAR4

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wehner, Michael

2005-07-08

SciDAC has invested heavily in climate change research. We offer a candid opinion as to the impact of the DOE laboratories' SciDAC projects on the upcoming Fourth Assessment Report of the Intergovernmental Panel on Climate Change. As a result of the direct importance of climate change to society, climate change research is highly coordinated at the international level. The Intergovernmental Panel on Climate Change (IPCC) is charged with providing regular reports on the state of climate change research to government policymakers. These reports are the product of thousands of scientists efforts. A series of reviews involving both scientists and policymakersmore » make them among the most reviewed documents produced in any scientific field. The high profile of these reports acts a driver to many researchers in the climate sciences. The Fourth Assessment Report (AR4) is scheduled to be released in 2007. SciDAC sponsored research has enabled the United States climate modeling community to make significant contributions to this report. Two large multi-Laboratory SciDAC projects are directly relevant to the activities of the IPCC. The first, entitled ''Collaborative Design and Development of the Community Climate System Model for Terascale Computers'', has made important software contributions to the recently released third version of the Community Climate System Model (CCSM3.0) developed at the National Center for Atmospheric Research. This is a multi-institutional project involving Los Alamos National Laboratory, Oak Ridge National Laboratory, Lawrence Berkeley National Laboratory, Pacific Northwest National Laboratory, Argonne National Laboratory, Lawrence Livermore National Laboratory and the National Center for Atmospheric Research. The original principal investigators were Robert Malone and John B. Drake. The current principal investigators are Phil Jones and John B. Drake. The second project, entitled ''Earth System Grid II: Turning Climate Datasets into Community Resources'' aims to facilitate the distribution of the copious amounts of data produced by coupled climate model integrations to the general scientific community. This is also a multi-institutional project involving Argonne National Laboratory, Oak Ridge National Laboratory, Lawrence Berkeley National Laboratory, Lawrence Livermore National Laboratory and the National Center for Atmospheric Research. The principal investigators are Ian Foster, Don Middleton and Dean Williams. Perhaps most significant among the activities of the ''Collaborative Design'', project was the development of an efficient multi-processor coupling package. CCSM3.0 is an extraordinarily complicated physics code. The fully coupled model consists of separate submodels of the atmosphere, ocean, sea ice and land. In addition, comprehensive biogeochemistry and atmospheric chemistry submodels are under intensive current development. Each of these submodels is a large and sophisticated program in its own right. Furthermore, in the coupled model, each of the submodels, including the coupler, is a separate multiprocessor executable program. The coupler package must efficiently coordinate the communication as well as interpolate or aggregate information between these programs. This regridding function is necessary because each major subsystem (air, water or surface) is allowed to have its own independent grid.« less

Integration of measurements with atmospheric dispersion models: Source term estimation for dispersal of (239)Pu due to non-nuclear detonation of high explosive

NASA Astrophysics Data System (ADS)

Edwards, L. L.; Harvey, T. F.; Freis, R. P.; Pitovranov, S. E.; Chernokozhin, E. V.

1992-10-01

The accuracy associated with assessing the environmental consequences of an accidental release of radioactivity is highly dependent on our knowledge of the source term characteristics and, in the case when the radioactivity is condensed on particles, the particle size distribution, all of which are generally poorly known. This paper reports on the development of a numerical technique that integrates the radiological measurements with atmospheric dispersion modeling. This results in a more accurate particle-size distribution and particle injection height estimation when compared with measurements of high explosive dispersal of (239)Pu. The estimation model is based on a non-linear least squares regression scheme coupled with the ARAC three-dimensional atmospheric dispersion models. The viability of the approach is evaluated by estimation of ADPIC model input parameters such as the ADPIC particle size mean aerodynamic diameter, the geometric standard deviation, and largest size. Additionally we estimate an optimal 'coupling coefficient' between the particles and an explosive cloud rise model. The experimental data are taken from the Clean Slate 1 field experiment conducted during 1963 at the Tonopah Test Range in Nevada. The regression technique optimizes the agreement between the measured and model predicted concentrations of (239)Pu by varying the model input parameters within their respective ranges of uncertainties. The technique generally estimated the measured concentrations within a factor of 1.5, with the worst estimate being within a factor of 5, very good in view of the complexity of the concentration measurements, the uncertainties associated with the meteorological data, and the limitations of the models. The best fit also suggest a smaller mean diameter and a smaller geometric standard deviation on the particle size as well as a slightly weaker particle to cloud coupling than previously reported.

Vitrification of radioactive high-level waste by spray calcination and in-can melting

NASA Astrophysics Data System (ADS)

Hanson, M. S.; Bjorklund, W. J.

1980-07-01

After several nonradioactive test runs, radioactive waste from the processing of 1.5 t of spent, light water reactor fuel was successfully concentrated, dried and converted to a vitreous product. A total of 97 L of waste glass (in two stainless steel canisters) was produced. The spray calcination process coupled to the in-can melting process, as developed at Pacific Northwest Labortory, was used to vitrify the waste. An effluent system consisting of a variety of condensation of scrubbing steps more than adequately decontaminated the process off gas before it was released to the atmosphere.

Regional Features and Seasonality of Land-Atmosphere Coupling over Eastern China

NASA Astrophysics Data System (ADS)

Gao, Chujie; Chen, Haishan; Sun, Shanlei; Xu, Bei; Ongoma, Victor; Zhu, Siguang; Ma, Hedi; Li, Xing

2018-06-01

Land-atmosphere coupling is a key process of the climate system, and various coupling mechanisms have been proposed before based on observational and numerical analyses. The impact of soil moisture (SM) on evapotranspiration (ET) and further surface temperature (ST) is an important aspect of such coupling. Using ERA-Interim data and CLM4.0 offline simulation results, this study further explores the relationships between SM/ST and ET to better understand the complex nature of the land-atmosphere coupling (i.e., spatial and seasonal variations) in eastern China, a typical monsoon area. It is found that two diagnostics of land-atmosphere coupling (i.e., SM-ET correlation and ST-ET correlation) are highly dependent on the climatology of SM and ST. By combining the SM-ET and ST-ET relationships, two "hot spots" of land-atmosphere coupling over eastern China are identified: Southwest China and North China. In Southwest China, ST is relatively high throughout the year, but SM is lowest in spring, resulting in a strong coupling in spring. However, in North China, SM is relatively low throughout the year, but ST is highest in summer, which leads to the strongest coupling in summer. Our results emphasize the dependence of land-atmosphere coupling on the seasonal evolution of climatic conditions and have implications for future studies related to land surface feedbacks.

Atmosphere-ocean feedbacks in a coastal upwelling system

NASA Astrophysics Data System (ADS)

Alves, J. M. R.; Peliz, A.; Caldeira, R. M. A.; Miranda, P. M. A.

2018-03-01

The COAWST (Coupled Ocean-Atmosphere-Wave-Sediment Transport) modelling system is used in different configurations to simulate the Iberian upwelling during the 2012 summer, aiming to assess the atmosphere-ocean feedbacks in the upwelling dynamics. When model results are compared with satellite measurements and in-situ data, two-way coupling is found to have a moderate impact in data-model statistics. A significant reinforcement of atmosphere-ocean coupling coefficients is, however, observed in the two-way coupled run, and in the WRF and ROMS runs forced by previously simulated SST and wind fields, respectively. The increasing in the coupling coefficient is associated with slight, but potentially important changes in the low-level coastal jet in the atmospheric marine boundary layer. While these results do not imply the need for fully coupled simulations in many applications, they show that in seasonal numerical studies such simulations do not degrade the overall model performance, and contribute to produce better dynamical fields.

Ocean-Atmosphere Coupled Model Simulations of Precipitation in the Central Andes

NASA Technical Reports Server (NTRS)

Nicholls, Stephen D.; Mohr, Karen I.

2015-01-01

The meridional extent and complex orography of the South American continent contributes to a wide diversity of climate regimes ranging from hyper-arid deserts to tropical rainforests to sub-polar highland regions. In addition, South American meteorology and climate are also made further complicated by ENSO, a powerful coupled ocean-atmosphere phenomenon. Modelling studies in this region have typically resorted to either atmospheric mesoscale or atmosphere-ocean coupled global climate models. The latter offers full physics and high spatial resolution, but it is computationally inefficient typically lack an interactive ocean, whereas the former offers high computational efficiency and ocean-atmosphere coupling, but it lacks adequate spatial and temporal resolution to adequate resolve the complex orography and explicitly simulate precipitation. Explicit simulation of precipitation is vital in the Central Andes where rainfall rates are light (0.5-5 mm hr-1), there is strong seasonality, and most precipitation is associated with weak mesoscale-organized convection. Recent increases in both computational power and model development have led to the advent of coupled ocean-atmosphere mesoscale models for both weather and climate study applications. These modelling systems, while computationally expensive, include two-way ocean-atmosphere coupling, high resolution, and explicit simulation of precipitation. In this study, we use the Coupled Ocean-Atmosphere-Wave-Sediment Transport (COAWST), a fully-coupled mesoscale atmosphere-ocean modeling system. Previous work has shown COAWST to reasonably simulate the entire 2003-2004 wet season (Dec-Feb) as validated against both satellite and model analysis data when ECMWF interim analysis data were used for boundary conditions on a 27-9-km grid configuration (Outer grid extent: 60.4S to 17.7N and 118.6W to 17.4W).

Composition and method for storing and releasing hydrogen

DOEpatents

Thorn, David L.; Tumas, William; Ott, Kevin C.; Burrell, Anthony K.

2010-06-15

A chemical system for storing and releasing hydrogen utilizes an endothermic reaction that releases hydrogen coupled to an exothermic reaction to drive the process thermodynamically, or an exothermic reaction that releases hydrogen coupled to an endothermic reaction.

Source Term Estimates of Radioxenon Released from the BaTek Medical Isotope Production Facility Using External Measured Air Concentrations

DOE Office of Scientific and Technical Information (OSTI.GOV)

Eslinger, Paul W.; Cameron, Ian M.; Dumais, Johannes R.

2015-10-01

Abstract Batan Teknologi (BaTek) operates an isotope production facility in Serpong, Indonesia that supplies 99mTc for use in medical procedures. Atmospheric releases of Xe-133 in the production process at BaTek are known to influence the measurements taken at the closest stations of the International Monitoring System (IMS). The purpose of the IMS is to detect evidence of nuclear explosions, including atmospheric releases of radionuclides. The xenon isotopes released from BaTek are the same as those produced in a nuclear explosion, but the isotopic ratios are different. Knowledge of the magnitude of releases from the isotope production facility helps inform analystsmore » trying to decide whether a specific measurement result came from a nuclear explosion. A stack monitor deployed at BaTek in 2013 measured releases to the atmosphere for several isotopes. The facility operates on a weekly cycle, and the stack data for June 15-21, 2013 show a release of 1.84E13 Bq of Xe-133. Concentrations of Xe-133 in the air are available at the same time from a xenon sampler located 14 km from BaTek. An optimization process using atmospheric transport modeling and the sampler air concentrations produced a release estimate of 1.88E13 Bq. The same optimization process yielded a release estimate of 1.70E13 Bq for a different week in 2012. The stack release value and the two optimized estimates are all within 10 percent of each other. Weekly release estimates of 1.8E13 Bq and a 40 percent facility operation rate yields a rough annual release estimate of 3.7E13 Bq of Xe-133. This value is consistent with previously published estimates of annual releases for this facility, which are based on measurements at three IMS stations. These multiple lines of evidence cross-validate the stack release estimates and the release estimates from atmospheric samplers.« less

Exploring coupled 4D-Var data assimilation using an idealised atmosphere-ocean model

NASA Astrophysics Data System (ADS)

Smith, Polly; Fowler, Alison; Lawless, Amos; Haines, Keith

2014-05-01

The successful application of data assimilation techniques to operational numerical weather prediction and ocean forecasting systems has led to an increased interest in their use for the initialisation of coupled atmosphere-ocean models in prediction on seasonal to decadal timescales. Coupled data assimilation presents a significant challenge but offers a long list of potential benefits including improved use of near-surface observations, reduction of initialisation shocks in coupled forecasts, and generation of a consistent system state for the initialisation of coupled forecasts across all timescales. In this work we explore some of the fundamental questions in the design of coupled data assimilation systems within the context of an idealised one-dimensional coupled atmosphere-ocean model. The system is based on the European Centre for Medium-Range Weather Forecasts (ECMWF) Integrated Forecast System (IFS) atmosphere model and a K-Profile Parameterisation (KKP) mixed layer ocean model developed by the National Centre for Atmospheric Science (NCAS) climate group at the University of Reading. It employs a strong constraint incremental 4D-Var scheme and is designed to enable the effective exploration of various approaches to performing coupled model data assimilation whilst avoiding many of the issues associated with more complex models. Working with this simple framework enables a greater range and quantity of experiments to be performed. Here, we will describe the development of our simplified single-column coupled atmosphere-ocean 4D-Var assimilation system and present preliminary results from a series of identical twin experiments devised to investigate and compare the behaviour and sensitivities of different coupled data assimilation methodologies. This includes comparing fully and weakly coupled assimilations with uncoupled assimilation, investigating whether coupled assimilation can eliminate or lessen initialisation shock in coupled model forecasts, and exploring the effect of the assimilation window length in coupled assimilations. These experiments will facilitate a greater theoretical understanding of the coupled atmosphere-ocean data assimilation problem and thus help guide the design and implementation of different coupling strategies within operational systems. This research is funded by the European Space Agency (ESA) and the UK Natural Environment Research Council (NERC). The ESA funded component is part of the Data Assimilation Projects - Coupled Model Data Assimilation initiative whose goal is to advance data assimilation techniques in fully coupled atmosphere-ocean models (see http://www.esa-da.org/). It is being conducted in parallel to the development of prototype weakly coupled data assimilation systems at both the UK Met Office and ECMWF.

The use of coupled atmospheric and hydrological models for water-resources management in headwater basins

USGS Publications Warehouse

Leavesley, G.; Hay, L.

1998-01-01

Coupled atmospheric and hydrological models provide an opportunity for the improved management of water resources in headwater basins. Issues currently limiting full implementation of coupled-model methodologies include (a) the degree of uncertainty in the accuracy of precipitation and other meteorological variables simulated by atmospheric models, and (b) the problem of discordant scales between atmospheric and bydrological models. Alternative methodologies being developed to address these issues are reviewed.

The Met Office Coupled Atmosphere/Land/Ocean/Sea-Ice Data Assimilation System

NASA Astrophysics Data System (ADS)

Lea, Daniel; Mirouze, Isabelle; Martin, Matthew; Hines, Adrian; Guiavarch, Catherine; Shelly, Ann

2014-05-01

The Met Office has developed a weakly-coupled data assimilation (DA) system using the global coupled model HADGEM3 (Hadley Centre Global Environment Model, version 3). This model combines the atmospheric model UM (Unified Model) at 60 km horizontal resolution on 85 vertical levels, the ocean model NEMO (Nucleus for European Modeling of the Ocean) at 25 km (at the equator) horizontal resolution on 75 vertical levels, and the sea-ice model CICE at the same resolution as NEMO. The atmosphere and the ocean/sea-ice fields are coupled every 1-hour using the OASIS coupler. The coupled model is corrected using two separate 6-hour window data assimilation systems: a 4D-Var for the atmosphere with associated soil moisture content nudging and snow analysis schemes on the one hand, and a 3D-Var FGAT for the ocean and sea-ice on the other hand. The background information in the DA systems comes from a previous 6-hour forecast of the coupled model. To show the impact of coupled DA, one-month experiments have been carried out, including 1) a full atmosphere/land/ocean/sea-ice coupled DA run, 2) an atmosphere-only run forced by OSTIA SSTs and sea-ice with atmosphere and land DA, and 3) an ocean-only run forced by atmospheric fields from run 2 with ocean and sea-ice DA. In addition, 5-day forecast runs, started twice a day, have been produced from initial conditions generated by either run 1 or a combination of runs 2 and 3. The different results have been compared to each other and, whenever possible, to other references such as the Met Office atmosphere and ocean operational analyses or the OSTIA data. These all show the coupled DA system functioning well. Evidence of imbalances and initialisation shocks has also been looked for.

Impact of two-way ocean atmosphere coupling on precipitation forecast for the coastal Adriatic region

NASA Astrophysics Data System (ADS)

Smerkol, Peter; Cedilnik, Jure; Fettich, Anja; Licer, Matjaz; Strajnar, Benedikt; Jerman, Jure

2017-04-01

A two-way coupled ocean and atmosphere modeling system has been developed at Slovenian Environment Agency and the National Institute of Biology (Ličer at al., 2016). The system comprises 4.4 km ALADIN/ALARO limited-area numerical weather prediction model and Princeton Ocean Model (POM) for Adriatic sea and uses Mediterranean Forecasting System (MFS) as ocean component outside the POM model domain. The heat and momentum fluxes between sea surface and atmosphere as estimated by ALADIN model are transferred into POM every model time stamp, and sea surface temperature (SST) is returned from POM to ALADIN. A positive impact of such a coupling system with respect to one-way coupling was demonstrated mainly for sea surface variables. In this contribution we study the impact on atmospheric variables, mainly precipitation. Unlike in the previous work where the atmospheric part of the system was reinitialized every day from external (non-coupled) data assimilation cycle, we implement the two-way coupling in the data assimilation cycle for ALADIN. Rather than running long-term simulations which would presumably lack observational information given no data assimilation for the ocean component, we focus on several precipitation events and assess performance of the atmospheric model by running the coupled system for a short warm-up periods beforehand the events. We evaluate several approaches to applying the one- or two-way coupling (in the warm-up period, during the main forecast, or both) and several approaches to using SST information in ALADIN in the one-way coupled mode (POM, MFS, global atmospheric model). Preliminary results suggest that it is important that two-way coupling is applied not only during the long term (e.g. 72 h) forecast but also already in the data assimilation cycle prior to event.

Harvesting Water from Air: Using Anhydrous Salt with Sunlight.

PubMed

Li, Renyuan; Shi, Yusuf; Shi, Le; Alsaedi, Mossab; Wang, Peng

2018-05-01

Atmospheric water is an abundant alternative water resource, equivalent to 6 times the water in all rivers on Earth. This work screens 14 common anhydrous and hydrated salt couples in terms of their physical and chemical stability, water vapor harvesting, and release capacity under relevant application scenarios. Among the salts screened, copper chloride (CuCl 2 ), copper sulfate (CuSO 4 ), and magnesium sulfate (MgSO 4 ) distinguish themselves and are further made into bilayer water collection devices, with the top layer being the photothermal layer, while the bottom layer acts as a salt-loaded fibrous membrane. The water collection devices are capable of capturing water vapor out of the air with low relative humidity (down to 15%) and releasing water under regular and even weakened sunlight (i.e., 0.7 kW/m 2 ). The work shines light on the potential use of anhydrous salt toward producing drinking water in water scarce regions.

Global Effects of SuperParameterization on Hydro-Thermal Land-Atmosphere Coupling on Multiple Timescales and an Amplification of the Bowen Ratio

NASA Astrophysics Data System (ADS)

Qin, H.; Pritchard, M. S.; Kooperman, G. J.; Parishani, H.

2017-12-01

Conventional General Circulation Models (GCMs) in the Global Land-Atmosphere Coupling Experiment (GLACE) tend to produce overly strong Land-Atmosphere coupling (L-A coupling) strength. We investigate the effects of cloud SuperParameterization (SP) on L-A coupling on timescales longer than the diurnal where it has been previously shown to have a strong effect. Using the Community Atmosphere Model v3.5 (CAM3.5) and its SuperParameterized counterpart SPCAM3.5, we conducted experiments following the GLACE and Atmospheric Model Intercomparison Project (AMIP) protocols. On synoptic-to-subseasonal timescales, SP significantly mutes hydrologic L-A coupling on a global scale, through the atmospheric segment. But on longer seasonal timescales, SP does not exhibit detectable effects on hydrologic L-A coupling. Two regional effects of SP on thermal L-A coupling are also discovered and explored. Over the Arabian Peninsula, SP strikingly reduces thermal L-A coupling due to a control by mean regional rainfall reduction. Over the Southwestern US and Northern Mexico, however, SP remarkably enhances the thermal L-A coupling independent of rainfall or soil moisture. We argue that the cause may be a previously unrecognized effect of SP to amplify the simulated Bowen ratio. Not only does this help reconcile a puzzling local enhancement of thermal L-A coupling over the Southwestern US, but it is also demonstrated to be a robust, global effect of SP over land that is independent of model version and experiment design, and that has important consequences for climate change prediction.

Large impacts and the evolution of Venus; an atmosphere/mantle coupled model.

NASA Astrophysics Data System (ADS)

Gillmann, Cedric; Tackley, Paul; Golabek, Gregor

2014-05-01

We investigate the evolution of atmosphere and surface conditions on Venus through a coupled model of mantle/atmosphere evolution by including meteoritic impacts mechanisms. Our main focuses are mechanisms that deplete or replenish the atmosphere: volcanic degassing, atmospheric escape and impacts. The coupling is obtained using feedback of the atmosphere on the mantle evolution. Atmospheric escape modeling involves two different aspects: hydrodynamic escape (dominant during the first few hundred million years) and non-thermal escape mechanisms as observed by the ASPERA instrument. Post 4 Ga escape is low. The atmosphere is replenished by volcanic degassing, using an adapted version of the StagYY mantle dynamics model (Armann and Tackley, 2012) and including episodic lithospheric overturn. Volatile fluxes are estimated for different mantle compositions and partitioning ratios. The evolving surface temperature is calculated from CO2 and water in the atmosphere with a gray radiative-convective atmosphere model. This surface temperature in turn acts as a boundary condition for the mantle dynamics model and has an influence on the convection, volcanism and subsequent degassing. We take into account the effects of meteorites in our simulations by adapting each relevant part of the model. They can bring volatiles as well as erode the atmosphere. Mantle dynamics are modified since the impact itself can also bring large amounts of energy to the mantle. A 2D distribution of the thermal anomaly due to the impact is used and can lead to melting. Volatile evolution due to impacts (especially the large ones) is heavily debated so we test a broad range of impactor parameters (size, velocity, timing) and test different assumptions related to impact erosion going from large eroding power (Ahrens 1993) to recent parameterization (Shuvalov, 2009, 2010). We are able to produce models leading to present-day-like conditions through episodic volcanic activity consistent with Venus observations. Without any impact, CO2 pressure only slightly increases due to degassing. On the other hand, water pressure varies rapidly leading to variations in surface temperatures of up to 200K, which have been identified to have an effect on volcanic activity. We observe a clear correlation between low temperature and mobile lid regime. We observe short term and long term effects of the impacts on planetary evolution. While small (less than kilometer scale) meteorites have a negligible effect, large ones (up to around 100 km) are able to bring volatiles to the planet and generate melt both at the impact and later on, due to volcanic events they triggered due to the changes they make to mantle dynamics. A significant amount of volatiles can be released on a short timescale. Depending on the timing of the impact, this can have significant long term effects on the surface condition evolution. Atmospheric erosion caused by impacts, on the other hand, and according to recent studies seems to have a marginal effect on the simulations, although the effects of the largest impactors is still debatable.

Source term estimates of radioxenon released from the BaTek medical isotope production facility using external measured air concentrations.

PubMed

Eslinger, Paul W; Cameron, Ian M; Dumais, Johannes Robert; Imardjoko, Yudi; Marsoem, Pujadi; McIntyre, Justin I; Miley, Harry S; Stoehlker, Ulrich; Widodo, Susilo; Woods, Vincent T

2015-10-01

BATAN Teknologi (BaTek) operates an isotope production facility in Serpong, Indonesia that supplies (99m)Tc for use in medical procedures. Atmospheric releases of (133)Xe in the production process at BaTek are known to influence the measurements taken at the closest stations of the radionuclide network of the International Monitoring System (IMS). The purpose of the IMS is to detect evidence of nuclear explosions, including atmospheric releases of radionuclides. The major xenon isotopes released from BaTek are also produced in a nuclear explosion, but the isotopic ratios are different. Knowledge of the magnitude of releases from the isotope production facility helps inform analysts trying to decide if a specific measurement result could have originated from a nuclear explosion. A stack monitor deployed at BaTek in 2013 measured releases to the atmosphere for several isotopes. The facility operates on a weekly cycle, and the stack data for June 15-21, 2013 show a release of 1.84 × 10(13) Bq of (133)Xe. Concentrations of (133)Xe in the air are available at the same time from a xenon sampler located 14 km from BaTek. An optimization process using atmospheric transport modeling and the sampler air concentrations produced a release estimate of 1.88 × 10(13) Bq. The same optimization process yielded a release estimate of 1.70 × 10(13) Bq for a different week in 2012. The stack release value and the two optimized estimates are all within 10% of each other. Unpublished production data and the release estimate from June 2013 yield a rough annual release estimate of 8 × 10(14) Bq of (133)Xe in 2014. These multiple lines of evidence cross-validate the stack release estimates and the release estimates based on atmospheric samplers. Copyright © 2015 Elsevier Ltd. All rights reserved.

Initial conditions and ENSO prediction using a coupled ocean-atmosphere model

NASA Astrophysics Data System (ADS)

Larow, T. E.; Krishnamurti, T. N.

1998-01-01

A coupled ocean-atmosphere initialization scheme using Newtonian relaxation has been developed for the Florida State University coupled ocean-atmosphere global general circulation model. The initialization scheme is used to initialize the coupled model for seasonal forecasting the boreal summers of 1987 and 1988. The atmosphere model is a modified version of the Florida State University global spectral model, resolution T-42. The ocean general circulation model consists of a slightly modified version of the Hamburg's climate group model described in Latif (1987) and Latif et al. (1993). The coupling is synchronous with information exchanged every two model hours. Using ECMWF atmospheric daily analysis and observed monthly mean SSTs, two, 1-year, time-dependent, Newtonian relaxation were performed using the coupled model prior to conducting the seasonal forecasts. The coupled initializations were conducted from 1 June 1986 to 1 June 1987 and from 1 June 1987 to 1 June 1988. Newtonian relaxation was applied to the prognostic atmospheric vorticity, divergence, temperature and dew point depression equations. In the ocean model the relaxation was applied to the surface temperature. Two, 10-member ensemble integrations were conducted to examine the impact of the coupled initialization on the seasonal forecasts. The initial conditions used for the ensembles are the ocean's final state after the initialization and the atmospheric initial conditions are ECMWF analysis. Examination of the SST root mean square error and anomaly correlations between observed and forecasted SSTs in the Niño-3 and Niño-4 regions for the 2 seasonal forecasts, show closer agreement between the initialized forecast than two, 10-member non-initialized ensemble forecasts. The main conclusion here is that a single forecast with the coupled initialization outperforms, in SST anomaly prediction, against each of the control forecasts (members of the ensemble) which do not include such an initialization, indicating possible importance for the inclusion of the atmosphere during the coupled initialization.

The Jet Stream's Precursor of M7.7 Russia Earthquake on 2017/07/17

NASA Astrophysics Data System (ADS)

Wu, H. C.

2017-12-01

Before M>6.0 earthquakes occurred, jet stream in the epicenter area will interrupt or velocity flow lines cross. That meaning is that before earthquake happen, atmospheric pressure in high altitude suddenly dropped during 6 12 hours (Wu & Tikhonov, 2014; Wu et.al,2015). The 70 knots speed line in jet stream was crossed at the epicenter on 2017/07/13, and then M7.7 Russia earthquake happened on 2017/07/17. Lithosphere-atmosphere-ionosphere (LAI) coupling model may be explained this phenomenon : Ionization of the air produced by an increased emanation of radon at epicenter. The water molecules in the air react with these ions, and then release heat. The heat result in temperature rise and pressure drop in the air(Pulinets, Ouzounov, 2011), and then the speed line of jet stream was changed. ps.Russia earthquake:M7.7 2017-07-17 23:34:13 (UTC) 54.471°N 168.815°E 11.0 kmReference: H.C Wu, I.N. Tikhonov, 2014, "Jet streams anomalies as possible short-term precursors of earthquakes with M>6.0", Research in geophysics. H.C.Wu., Ivan N. Tikhonov, and Ariel R. Ćesped,2015, Multi-parametric analysis of earthquake precursors, Russ. J. Earth. Sci., 15, ES3002, doi:10.2205/2015ES000553 S Pulinets, D Ouzounov, 2011,"Lithosphere-Atmosphere-Ionosphere Coupling (LAIC) model-An unified concept for earthquake precursors validation", Journal of Asian Earth Sciences 41 (4), 371-382.

Land-atmosphere coupling manifested in warm-season observations on the U.S. southern great plains

DOE PAGES

Phillips, Thomas J.; Klein, Stephen A.

2014-01-28

This study examines several observational aspects of land-atmosphere coupling on daily average time scales during warm seasons of the years 1997 to 2008 at the Department of Energy Atmospheric Radiation Measurement Program’s Southern Great Plains (SGP) Central Facility site near Lamont, Oklahoma. Characteristics of the local land-atmosphere coupling are inferred by analyzing the covariability of selected land and atmospheric variables that include precipitation and soil moisture, surface air temperature, relative humidity, radiant and turbulent fluxes, as well as low-level cloud base height and fractional coverage. For both the energetic and hydrological aspects of this coupling, it is found that large-scalemore » atmospheric forcings predominate, with local feedbacks of the land on the atmosphere being comparatively small much of the time. The weak land feedbacks are manifested by 1) the inability of soil moisture to comprehensively impact the coupled land-atmosphere energetics, and 2) the limited recycling of local surface moisture under conditions where most of the rainfall derives from convective cells that originate at remote locations. There is some evidence, nevertheless, of the local land feedback becoming stronger as the soil dries out in the aftermath of precipitation events, or on days when the local boundary-layer clouds are influenced by thermal updrafts known to be associated with convection originating at the surface. Finally, we also discuss potential implications of these results for climate-model representation of regional land-atmosphere coupling.« less

Land-atmosphere coupling and soil moisture memory contribute to long-term agricultural drought

NASA Astrophysics Data System (ADS)

Kumar, S.; Newman, M.; Lawrence, D. M.; Livneh, B.; Lombardozzi, D. L.

2017-12-01

We assessed the contribution of land-atmosphere coupling and soil moisture memory on long-term agricultural droughts in the US. We performed an ensemble of climate model simulations to study soil moisture dynamics under two atmospheric forcing scenarios: active and muted land-atmosphere coupling. Land-atmosphere coupling contributes to a 12% increase and 36% decrease in the decorrelation time scale of soil moisture anomalies in the US Great Plains and the Southwest, respectively. These differences in soil moisture memory affect the length and severity of modeled drought. Consequently, long-term droughts are 10% longer and 3% more severe in the Great Plains, and 15% shorter and 21% less severe in the Southwest. An analysis of Coupled Model Intercomparsion Project phase 5 data shows four fold uncertainty in soil moisture memory across models that strongly affects simulated long-term droughts and is potentially attributable to the differences in soil water storage capacity across models.

Methyl tert‐butyl ether degradation in the unsaturated zone and the relation between MTBE in the atmosphere and shallow groundwater

USGS Publications Warehouse

Baehr, Arthur L.; Charles, Emmanuel G.; Baker, Ronald J.

2001-01-01

Atmospheric methyl tert‐butyl ether (MTBE) concentrations in southern New Jersey generally exceeded concentrations in samples taken from the unsaturated zone. A simple unsaturated zone transport model indicates that MTBE degradation can explain the attenuation with half‐lives from a few months to a couple of years. Tert‐butyl alcohol (TBA), a possible degradation product of MTBE, was detected in unsaturated‐zone samples at concentrations exceeding atmospheric levels at some sites, suggesting the possible conversion of MTBE to TBA. At sites where MTBE was detected in shallow groundwater, the concentration was typically higher than the overlying unsaturated‐zone concentration. This observation is consistent with outgassing from the aquifer and combined with the unsaturated‐zone attenuation suggests some of the MTBE detections in shallow groundwater are nonatmospheric in origin, coming from leaking tanks, road runoff, or other sources. The identification of sources of MTBE in groundwater and attenuation mechanisms through the hydrologic cycle is critical in developing an understanding of the long‐term effect of MTBE releases.

The Numerical Simulation of a Tracer-Release Field Project to Study Motion within the Nocturnal Boundary Layer

NASA Astrophysics Data System (ADS)

Werth, D. W.; Leclerc, M. Y.; Buckley, R.; Parker, M.; Kurzeja, R.; Duarte, H. F.; Zhang, G.; Durden, D.

2009-12-01

The Savannah River National Laboratory (SRNL), Brookhaven National Laboratory (BNL), the University of Georgia (UGA), and the National Oceanic and Atmospheric Administration (NOAA) conducted a regional tracer experiment to study the nocturnal behavior of CO2 in the vicinity of an instrumented tall tower during two nights on May 11th and 12th, 2009. The experiment consisted of a release of five perfluorocarbon tracer (PFTs) compounds in twelve unique locations in Aiken County, South Carolina. Intensive meteorological measurements including in-situ turbulence were made in conjunction with the release and sampling of the PFTs. A 300m tower was also used to collect data from higher levels, allowing us to determine the extent to which the tracer was mixed vertically. Lagrangian plume simulations performed during the experiment demonstrated transport over distances of >8 km, and correlated well with in situ sampling. The area was characterized by heavy vegetation cover, and carbon dioxide concentrations were also monitored in an effort to determine how respiration and advection affect CO2 levels in the stable layer. Tracer release locations were carefully selected via a fine-scale mesoscale modeling study of similar nights. The purpose of these experiments was to provide data that will be used to increase the understanding of the terrestrial carbon budget, especially with respect to nocturnal boundary layer (NBL) phenomena such as low level jets and breaking gravity waves. Using these data, a simulation of the motion of the tracer within the boundary layer was developed using the Regional Atmospheric Modeling System (RAMS) mesoscale model coupled to a tracer model. The RAMS model was also coupled to the Simple Biosphere (SiB) vegetation model, which allowed for the simulation of the release of carbon dioxide into the NBL. The simulation results are used to validate the NBL hypothesis of CO2 monitoring, by which the release of CO2 can be correlated with the accumulation of CO2 in the boundary layer beneath a stable ‘lid’, which impedes vertical mixing. This is done with both the tracer, in which the release rate is known and no advection occurs, and for CO2, in which the release rate is not known and for which advection of CO2 must be accounted. The high resolution of the simulation allows us to resolve the small-scale motions within the NBL, which are important to nocturnal transport. Flux data from the tall tower were studied to learn more about the eddy transport, and also to detect the occurrence of transport ‘events’ in which the CO2 and H2O values experience a sudden increase. A wavelet analysis is also applied, and reveals the existence of eddy activity dominated by eddies of diameter 90-240m.

Estimates of Radioxenon Released from Southern Hemisphere Medical isotope Production Facilities Using Measured Air Concentrations and Atmospheric Transport Modeling

DOE Office of Scientific and Technical Information (OSTI.GOV)

Eslinger, Paul W.; Friese, Judah I.; Lowrey, Justin D.

2014-09-01

Abstract The International Monitoring System (IMS) of the Comprehensive-Nuclear-Test-Ban-Treaty monitors the atmosphere for radioactive xenon leaking from underground nuclear explosions. Emissions from medical isotope production represent a challenging background signal when determining whether measured radioxenon in the atmosphere is associated with a nuclear explosion prohibited by the treaty. The Australian Nuclear Science and Technology Organisation (ANSTO) operates a reactor and medical isotope production facility in Lucas Heights, Australia. This study uses two years of release data from the ANSTO medical isotope production facility and Xe-133 data from three IMS sampling locations to estimate the annual releases of Xe-133 from medicalmore » isotope production facilities in Argentina, South Africa, and Indonesia. Atmospheric dilution factors derived from a global atmospheric transport model were used in an optimization scheme to estimate annual release values by facility. The annual releases of about 6.8×1014 Bq from the ANSTO medical isotope production facility are in good agreement with the sampled concentrations at these three IMS sampling locations. Annual release estimates for the facility in South Africa vary from 1.2×1016 to 2.5×1016 Bq and estimates for the facility in Indonesia vary from 6.1×1013 to 3.6×1014 Bq. Although some releases from the facility in Argentina may reach these IMS sampling locations, the solution to the objective function is insensitive to the magnitude of those releases.« less

A sulfur hexafluoride sensor using quantum cascade and CO2 laser-based photoacoustic spectroscopy.

PubMed

Rocha, Mila; Sthel, Marcelo; Lima, Guilherme; da Silva, Marcelo; Schramm, Delson; Miklós, András; Vargas, Helion

2010-01-01

The increase in greenhouse gas emissions is a serious environmental problem and has stimulated the scientific community to pay attention to the need for detection and monitoring of gases released into the atmosphere. In this regard, the development of sensitive and selective gas sensors has been the subject of several research programs. An important greenhouse gas is sulphur hexafluoride, an almost non-reactive gas widely employed in industrial processes worldwide. Indeed it is estimated that it has a radiative forcing of 0.52 W/m(2). This work compares two photoacoustic spectrometers, one coupled to a CO(2) laser and another one coupled to a Quantum Cascade (QC) laser, for the detection of SF(6). The laser photoacoustic spectrometers described in this work have been developed for gas detection at small concentrations. Detection limits of 20 ppbv for CO(2) laser and 50 ppbv for quantum cascade laser were obtained.

Numerical Modelling of Fire-Atmosphere Interactions and the 2003 Canberra Bushfires

NASA Astrophysics Data System (ADS)

Simpson, C.; Sturman, A.; Zawar-Reza, P.

2010-12-01

It is well known that the behaviour of a wildland fire is strongly associated with the conditions of its surrounding atmosphere. However, the two-way interactions between fire behaviour and the atmospheric conditions are not well understood. A numerical model is used to simulate wildland fires so that the nature of these fire-atmosphere interactions, and how they might affect fire behaviour, can be further investigated. The 2003 Canberra bushfires are used as a case study due to their highly destructive and unusual behaviour. On the 18th January 2003, these fires spread to the urban suburbs of Canberra, resulting in the loss of four lives and the destruction of over 500 homes. Fire-atmosphere interactions are believed to have played an important role in making these fires so destructive. WRF-Fire is used to perform real data simulations of the 2003 Canberra bushfires. WRF-Fire is a coupled fire-atmosphere model, which combines a semi-empirical fire spread model with an atmospheric model, allowing it to directly simulate the two-way interactions between a fire and its surrounding atmosphere. These simulations show the impact of the presence of a fire on conditions within the atmospheric boundary layer. This modification of the atmosphere, resulting from the injection of heat and moisture released by the fire, appears to have a direct feedback onto the overall fire behaviour. The bushfire simulations presented in this paper provide important scientific insights into the nature of fire-atmosphere interactions for a real situation. It is expected that they will also help fire managers in Australia to better understand why the 2003 Canberra bushfires were so destructive, as well as to gain improved insight into bushfire behaviour in general.

Numerical modeling of the effects of fire-induced convection and fire-atmosphere interactions on wildfire spread and fire plume dynamics

NASA Astrophysics Data System (ADS)

Sun, Ruiyu

It is possible due to present day computing power to produce a fluid dynamical physically-based numerical solution to wildfire behavior, at least in the research mode. This type of wildfire modeling affords a flexibility and produces details that are not available in either current operational wildfire behavior models or field experiments. However before using these models to study wildfire, validation is necessary, and model results need to be systematically and objectively analyzed and compared to real fires. Plume theory and data from the Meteotron experiment, which was specially designed to provide results from measurements for the theoretical study of a convective plume produced by a high heat source at the ground, are used here to evaluate the fire plume properties simulated by two numerical wildfire models, the Fire Dynamics Simulator or FDS, and the Clark coupled atmosphere-fire model. The study indicates that the FDS produces good agreement with the plume theory and the Meteotron results. The study also suggests that the coupled atmosphere-fire model, a less explicit and ideally less computationally demanding model than the FDS; can produce good agreement, but that the agreement is sensitive to the method of putting the energy released from the fire into the atmosphere. The WFDS (Wildfire and wildland-urban interface FDS), an extension of the FDS to the vegetative fuel, and the Australian grass fire experiments are used to evaluate and improve the UULES-wildfire coupled model. Despite the simple fire parameterization in the UULES-wildfire coupled model, the fireline is fairly well predicted in terms of both shape and location in the simulation of Australian grass fire experiment F19. Finally, the UULES-wildfire coupled model is used to examine how the turbulent flow in the atmospheric boundary layer (ABL) affects the growth of the grass fires. The model fires showed significant randomness in fire growth: Fire spread is not deterministic in the ABL, and a probabilistic prediction method is warranted. Of the two contributors to the variability in fire growth in the grass fire simulations in the ABL, fire-induced convection, as opposed to the turbulent ABL wind, appears to be the more important one. One mechanism associated with enhanced fire-induced flow is the downdraft behind the frontal fireline. The downdraft is the direct result of the random interaction between the fire plume and the large eddies in the ABL. This study indicates a connection between fire variability in rate of spread and area burnt and so-called convective velocity scale, and it may be possible to use this boundary-layer scale parameter to account for the effects of ABL turbulence on fire spread and fire behavior in today's operational fire prediction systems.

Towards a more detailed representation of the energy balance in a coupled land surface model

NASA Astrophysics Data System (ADS)

Ryder, J.; Polcher, J.; Luyssaert, S.

2012-04-01

Currently, the land-surface region sequesters 25% of global CO2 emissions. In addition to climate change, increasing atmospheric CO2 concentrations, fertilisation and nitrogen deposition, this sink is thought to be largely due to land management. When applied deliberately to enhance the terrestrial carbon sink strength, this land management may have unintended effects on the energy budget, potentially offsetting the radiative effect of carbon sequestration. As with other land surface models, the present release of ORCHIDEE (the land surface model of the IPSL Earth system model) has difficulties in reproducing consistently observed energy balances (Pitman et al., 2009; Jimenez et al., 2011; de Noblet-Ducoudré et al., 2011). Hence, the model must be improved to be better able to study the radiative effect of forest management and land use change. This observation serves as a starting point in this research - improving the level of detail in energy balance simulations of the surface layer. We here outline the structure of a new detailed and practical simulation of the energy budget that is currently under development within the surface model ORCHIDEE, and will be coupled to the atmospheric model LMDZ. The most detailed simulations of the surface layer energy budget are detailed iterative multi-layer canopy models, such as Ogeé et al. (2003), which are linked to specific measurement sites and do not interact with the atmosphere. In this current project, we aim to create a model that will implement the insights obtained in those previous studies and improve upon the present ORCHIDEE parameterisation, but will run stably and efficiently when coupled to an atmospheric model. This work involves a replacement of the existing allocation of 14 different types of vegetation within each surface tile (the 'Plant Functional Types') by a more granular scheme that can be modified to reflect changes in attributes such as vegetation density, leaf type, distribution (clumping factors), age and height of vegetation within the surface tile. There will be the implementation of more than one canopy vegetation layer to simulate the effects of scalar gradients within the canopy for determining, more accurately, the net sensible and latent heat fluxes that are passed to the atmosphere. The model will include representation of characteristics such as in-canopy transport, coupling with sensible heat flux from the soil, a multilayer radiation budget and stomatal resistance, and interaction with the bare soil flux within the canopy space (and also with snow pack). We present how the implicit coupling approach of Polcher et al. (1998) and Best et al. (2004) is to be extended to a multilayer scenario, present initial sensitivity studies and outline future testing scenarios and validation plans.

Collisionless coupling processes in AMPTE releases

NASA Technical Reports Server (NTRS)

Lui, A. T. Y.

1990-01-01

An evaluation is made of results obtained to date by in situ measurements, numerical simulations, and theoretical considerations of Active Magnetospheric Particle Tracer Explorer chemical releases bearing on the nature of collisionless coupling processes. It is noted that both laminar and turbulent forces act to couple the solar wind momentum and energy to the release cloud; the magnetic field compression formed in this interaction plays an important intermediary role in coupling the two plasmas, and the intense electrostatic turbulence generated enhances the interaction. A scenario accounting for several features in the observed evolution of the December 27, 1984 artificial comet release is presented.

MAVEN Contamination Venting and Outgassing Analysis

NASA Technical Reports Server (NTRS)

Petro, Elaine M.; Hughes, David W.; Secunda, Mark S.; Chen, Philip T.; Morrissey, James R.; Riegle, Catherine A.

2014-01-01

Mars Atmosphere and Volatile EvolutioN (MAVEN) is the first mission to focus its study on the Mars upper atmosphere. MAVEN will study the evolution of the Mars atmosphere and climate, by examining the conduit through which the atmosphere has to pass as it is lost to the upper atmosphere. An analysis was performed for the MAVEN mission to address two distinct concerns. The first goal of the analysis was to perform an outgassing study to determine where species outgassed from spacecraft materials would redistribute to and how much of the released material might accumulate on sensitive surfaces. The second portion of the analysis serves to predict what effect, if any, Mars atmospheric gases trapped within the spacecraft could have on instrument measurements when re-released through vents. The re-release of atmospheric gases is of interest to this mission because vented gases from a higher pressure spacecraft interior could bias instrument measurements of the Mars atmosphere depending on the flow rates and directions.

Using ARM Observations to Evaluate Climate Model Simulations of Land-Atmosphere Coupling on the U.S. Southern Great Plains

DOE Office of Scientific and Technical Information (OSTI.GOV)

Phillips, Thomas J.; Klein, Stephen A.; Ma, Hsi -Yen

Several independent measurements of warm-season soil moisture and surface atmospheric variables recorded at the ARM Southern Great Plains (SGP) research facility are used to estimate the terrestrial component of land-atmosphere coupling (LAC) strength and its regional uncertainty. The observations reveal substantial variation in coupling strength, as estimated from three soil moisture measurements at a single site, as well as across six other sites having varied soil and land cover types. The observational estimates then serve as references for evaluating SGP terrestrial coupling strength in the Community Atmospheric Model coupled to the Community Land Model. These coupled model components are operatedmore » in both a free-running mode and in a controlled configuration, where the atmospheric and land states are reinitialized daily, so that they do not drift very far from observations. Although the controlled simulation deviates less from the observed surface climate than its free-running counterpart, the terrestrial LAC in both configurations is much stronger and displays less spatial variability than the SGP observational estimates. Preliminary investigation of vegetation leaf area index (LAI) substituted for soil moisture suggests that the overly strong coupling between model soil moisture and surface atmospheric variables is associated with too much evaporation from bare ground and too little from the vegetation cover. Lastly, these results imply that model surface characteristics such as LAI, as well as the physical parameterizations involved in the coupling of the land and atmospheric components, are likely to be important sources of the problematical LAC behaviors.« less

Using ARM Observations to Evaluate Climate Model Simulations of Land-Atmosphere Coupling on the U.S. Southern Great Plains

DOE PAGES

Phillips, Thomas J.; Klein, Stephen A.; Ma, Hsi -Yen; ...

2017-10-13

Several independent measurements of warm-season soil moisture and surface atmospheric variables recorded at the ARM Southern Great Plains (SGP) research facility are used to estimate the terrestrial component of land-atmosphere coupling (LAC) strength and its regional uncertainty. The observations reveal substantial variation in coupling strength, as estimated from three soil moisture measurements at a single site, as well as across six other sites having varied soil and land cover types. The observational estimates then serve as references for evaluating SGP terrestrial coupling strength in the Community Atmospheric Model coupled to the Community Land Model. These coupled model components are operatedmore » in both a free-running mode and in a controlled configuration, where the atmospheric and land states are reinitialized daily, so that they do not drift very far from observations. Although the controlled simulation deviates less from the observed surface climate than its free-running counterpart, the terrestrial LAC in both configurations is much stronger and displays less spatial variability than the SGP observational estimates. Preliminary investigation of vegetation leaf area index (LAI) substituted for soil moisture suggests that the overly strong coupling between model soil moisture and surface atmospheric variables is associated with too much evaporation from bare ground and too little from the vegetation cover. Lastly, these results imply that model surface characteristics such as LAI, as well as the physical parameterizations involved in the coupling of the land and atmospheric components, are likely to be important sources of the problematical LAC behaviors.« less

Selective deuteration illuminates the importance of tunneling in the unimolecular decay of Criegee intermediates to hydroxyl radical products

DOE PAGES

Green, Amy M.; Barber, Victoria P.; Fang, Yi; ...

2017-11-06

Ozonolysis of alkenes, an important nonphotolytic source of hydroxyl (OH) radicals in the atmosphere, proceeds through unimolecular decay of Criegee intermediates. Here, we report a large kinetic isotope effect associated with the rate-limiting hydrogen-transfer step that releases OH radicals for a prototypical Criegee intermediate, CH 3CHOO. IR excitation of selectively deuterated syn-CD 3CHOO is shown to result in deuterium atom transfer and release OD radical products. Vibrational activation of syn-CD 3CHOO is coupled with direct time-resolved detection of OD products to measure a 10-fold slower rate of unimolecular decay upon deuteration in the vicinity of the transition state barrier, whichmore » is confirmed by microcanonical statistical theory that incorporates quantum mechanical tunneling. The corresponding kinetic isotope effect of ~10 is attributed primarily to the decreased probability of D-atom vs. H-atom transfer arising from tunneling. Master equation modeling is utilized to compute the thermal unimolecular decay rates for selectively and fully deuterated syn methyl-substituted Criegee intermediates under atmospheric conditions. Lastly, at 298 K (1 atm), tunneling is predicted to enhance the thermal decay rate of syn-CH 3CHOO compared with the deuterated species, giving rise to a significant kinetic isotope effect of ~50.« less

Selective deuteration illuminates the importance of tunneling in the unimolecular decay of Criegee intermediates to hydroxyl radical products

DOE Office of Scientific and Technical Information (OSTI.GOV)

Green, Amy M.; Barber, Victoria P.; Fang, Yi

Ozonolysis of alkenes, an important nonphotolytic source of hydroxyl (OH) radicals in the atmosphere, proceeds through unimolecular decay of Criegee intermediates. Here, we report a large kinetic isotope effect associated with the rate-limiting hydrogen-transfer step that releases OH radicals for a prototypical Criegee intermediate, CH 3CHOO. IR excitation of selectively deuterated syn-CD 3CHOO is shown to result in deuterium atom transfer and release OD radical products. Vibrational activation of syn-CD 3CHOO is coupled with direct time-resolved detection of OD products to measure a 10-fold slower rate of unimolecular decay upon deuteration in the vicinity of the transition state barrier, whichmore » is confirmed by microcanonical statistical theory that incorporates quantum mechanical tunneling. The corresponding kinetic isotope effect of ~10 is attributed primarily to the decreased probability of D-atom vs. H-atom transfer arising from tunneling. Master equation modeling is utilized to compute the thermal unimolecular decay rates for selectively and fully deuterated syn methyl-substituted Criegee intermediates under atmospheric conditions. Lastly, at 298 K (1 atm), tunneling is predicted to enhance the thermal decay rate of syn-CH 3CHOO compared with the deuterated species, giving rise to a significant kinetic isotope effect of ~50.« less

Selective deuteration illuminates the importance of tunneling in the unimolecular decay of Criegee intermediates to hydroxyl radical products.

PubMed

Green, Amy M; Barber, Victoria P; Fang, Yi; Klippenstein, Stephen J; Lester, Marsha I

2017-11-21

Ozonolysis of alkenes, an important nonphotolytic source of hydroxyl (OH) radicals in the atmosphere, proceeds through unimolecular decay of Criegee intermediates. Here, we report a large kinetic isotope effect associated with the rate-limiting hydrogen-transfer step that releases OH radicals for a prototypical Criegee intermediate, CH 3 CHOO. IR excitation of selectively deuterated syn -CD 3 CHOO is shown to result in deuterium atom transfer and release OD radical products. Vibrational activation of syn -CD 3 CHOO is coupled with direct time-resolved detection of OD products to measure a 10-fold slower rate of unimolecular decay upon deuteration in the vicinity of the transition state barrier, which is confirmed by microcanonical statistical theory that incorporates quantum mechanical tunneling. The corresponding kinetic isotope effect of ∼10 is attributed primarily to the decreased probability of D-atom vs. H-atom transfer arising from tunneling. Master equation modeling is utilized to compute the thermal unimolecular decay rates for selectively and fully deuterated syn methyl-substituted Criegee intermediates under atmospheric conditions. At 298 K (1 atm), tunneling is predicted to enhance the thermal decay rate of syn -CH 3 CHOO compared with the deuterated species, giving rise to a significant kinetic isotope effect of ∼50.

Selective deuteration illuminates the importance of tunneling in the unimolecular decay of Criegee intermediates to hydroxyl radical products

PubMed Central

Green, Amy M.; Barber, Victoria P.; Fang, Yi; Klippenstein, Stephen J.; Lester, Marsha I.

2017-01-01

Ozonolysis of alkenes, an important nonphotolytic source of hydroxyl (OH) radicals in the atmosphere, proceeds through unimolecular decay of Criegee intermediates. Here, we report a large kinetic isotope effect associated with the rate-limiting hydrogen-transfer step that releases OH radicals for a prototypical Criegee intermediate, CH3CHOO. IR excitation of selectively deuterated syn-CD3CHOO is shown to result in deuterium atom transfer and release OD radical products. Vibrational activation of syn-CD3CHOO is coupled with direct time-resolved detection of OD products to measure a 10-fold slower rate of unimolecular decay upon deuteration in the vicinity of the transition state barrier, which is confirmed by microcanonical statistical theory that incorporates quantum mechanical tunneling. The corresponding kinetic isotope effect of ∼10 is attributed primarily to the decreased probability of D-atom vs. H-atom transfer arising from tunneling. Master equation modeling is utilized to compute the thermal unimolecular decay rates for selectively and fully deuterated syn methyl-substituted Criegee intermediates under atmospheric conditions. At 298 K (1 atm), tunneling is predicted to enhance the thermal decay rate of syn-CH3CHOO compared with the deuterated species, giving rise to a significant kinetic isotope effect of ∼50. PMID:29109292

Using ARM Observations to Evaluate Climate Model Representation of Land-Atmosphere Coupling on the U.S. Southern Great Plains

NASA Astrophysics Data System (ADS)

Phillips, T. J.; Klein, S. A.; Ma, H. Y.; Tang, Q.

2016-12-01

Statistically significant coupling between summertime soil moisture and various atmospheric variables has been observed at the U.S. Southern Great Plains (SGP) facilities maintained by the U.S. DOE Atmospheric Radiation Measurement (ARM) program (Phillips and Klein, 2014 JGR). In the current study, we employ several independent measurements of shallow-depth soil moisture (SM) and of the surface evaporative fraction (EF) over multiple summers in order to estimate the range of SM-EF coupling strength at seven sites, and to approximate the SGP regional-scale coupling strength (and its uncertainty). We will use this estimate of regional-scale SM-EF coupling strength to evaluate its representation in version 5.1 of the global Community Atmosphere Model (CAM5.1) coupled to the CLM4 Land Model. Two experimental cases are considered for the 2003-2011 study period: 1) an Atmospheric Model Intercomparison Project (AMIP) run with historically observed sea surface temperatures specified, and 2) a more constrained hindcast run in which the CAM5.1 atmospheric state is initialized each day from the ERA Interim reanalysis, while the CLM4 initial conditions are obtained from an offline run of the land model using observed surface net radiation, precipitation, and wind as forcings. These twin experimental cases allow a distinction to be drawn between the land-atmosphere coupling in the free-running CAM5.1/CLM4 model and that in which the land and atmospheric states are constrained to remain closer to "reality". The constrained hindcast case, for example, should allow model errors in coupling strength to be related more closely to potential deficiencies in land-surface or atmospheric boundary-layer parameterizations. AcknowledgmentsThis work was funded by the U.S. Department of Energy Office of Science and was performed at the Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

Evaluation on chemical stability of lead blast furnace (LBF) and imperial smelting furnace (ISF) slags.

PubMed

Yin, Nang-Htay; Sivry, Yann; Guyot, François; Lens, Piet N L; van Hullebusch, Eric D

2016-09-15

The leaching behavior of Pb and Zn from lead blast furnace (LBF) and imperial smelting furnace (ISF) slags sampled in the North of France was studied as a function of pHs and under two atmospheres (open air and nitrogen). The leaching of major elements from the slags was monitored as a function of pH (4, 5.5, 7, 8.5 and 10) under both atmospheres for different slag-water interaction times (1 day and 9 days). The leaching results were coupled with a geochemical model; Visual MINTEQ version 3.0, and a detailed morphological and mineralogical analysis was performed on the leached slags by scanning and transmission electron microscopy (SEM and TEM). Significant amounts of Ca, Fe and Zn were released under acidic conditions (pH 4) with a decrease towards the neutral to alkaline conditions (pH 7 and 10) for both LBF and ISF slags. On the other hand, Fe leachability was limited at neutral to alkaline pH for both slags. The concentrations of all elements increased gradually after 216 h compared to initial 24 h of leaching period. The presence of oxygen under open-air atmosphere not only enhanced oxidative weathering but also encouraged formation of secondary oxide and carbonate phases. Formation of carbonates and clay minerals was suggested by Visual MINTEQ which was further confirmed by SEM & TEM. The hydration and partial dissolution of hardystonite, as well as the destabilization of amorphous glassy matrix mainly contributed to the release of major elements, whereas the spinel related oxides were resistant against pH changes and atmospheres within the time frame concerned for both LBF and ISF slags. The total amount of Pb leached out at pH 7 under both atmospheres suggested that both LBF and ISF slags are prone to weathering even at neutral environmental conditions. Copyright © 2016 Elsevier Ltd. All rights reserved.

Modulated Hawking radiation and a nonviolent channel for information release

DOE PAGES

Giddings, Steven B.

2014-09-16

The unitarization of black hole evaporation requires that quantum information escapes a black hole; an important question is to identify the mechanism or channel by which it does so. Accurate counting of black hole states via the Bekenstein–Hawking entropy would indicate this information should be encoded in radiation with average energy flux matching Hawking’s. Information can be encoded with no change in net flux via fine-grained modulation of the Hawking radiation. In an approximate effective field theory description, couplings to the stress tensor of the black hole atmosphere that depend on the internal state of the black hole are amore » promising alternative for inducing such modulation. These can be picturesquely thought of as due to state-dependent metric fluctuations in the vicinity of the horizon. Such couplings offer the prospect of emitting information without extra energy flux, and can be shown to do so at linear order in the couplings, with motivation given for possible extension of this result to higher orders. The potential advantages of such couplings to the stress tensor thus extend beyond their universality, which is helpful in addressing constraints from black hole mining.« less

Intercomparison of oceanic and atmospheric forced and coupled mesoscale simulations. Part I: Surface fluxes

NASA Astrophysics Data System (ADS)

Josse, P.; Caniaux, G.; Giordani, H.; Planton, S.

1999-04-01

A mesoscale non-hydrostatic atmospheric model has been coupled with a mesoscale oceanic model. The case study is a four-day simulation of a strong storm event observed during the SEMAPHORE experiment over a 500 × 500 km2 domain. This domain encompasses a thermohaline front associated with the Azores current. In order to analyze the effect of mesoscale coupling, three simulations are compared: the first one with the atmospheric model forced by realistic sea surface temperature analyses; the second one with the ocean model forced by atmospheric fields, derived from weather forecast re-analyses; the third one with the models being coupled. For these three simulations the surface fluxes were computed with the same bulk parametrization. All three simulations succeed well in representing the main oceanic or atmospheric features observed during the storm. Comparison of surface fields with in situ observations reveals that the winds of the fine mesh atmospheric model are more realistic than those of the weather forecast re-analyses. The low-level winds simulated with the atmospheric model in the forced and coupled simulations are appreciably stronger than the re-analyzed winds. They also generate stronger fluxes. The coupled simulation has the strongest surface heat fluxes: the difference in the net heat budget with the oceanic forced simulation reaches on average 50 Wm-2 over the simulation period. Sea surface-temperature cooling is too weak in both simulations, but is improved in the coupled run and matches better the cooling observed with drifters. The spatial distributions of sea surface-temperature cooling and surface fluxes are strongly inhomogeneous over the simulation domain. The amplitude of the flux variation is maximum in the coupled run. Moreover the weak correlation between the cooling and heat flux patterns indicates that the surface fluxes are not responsible for the whole cooling and suggests that the response of the ocean mixed layer to the atmosphere is highly non-local and enhanced in the coupled simulation.

Description and verification of a U.S. Naval Research Lab's loosely coupled data assimilation system for the Navy's Earth System Model

NASA Astrophysics Data System (ADS)

Barton, N. P.; Metzger, E. J.; Smedstad, O. M.; Ruston, B. C.; Wallcraft, A. J.; Whitcomb, T.; Ridout, J. A.; Zamudio, L.; Posey, P.; Reynolds, C. A.; Richman, J. G.; Phelps, M.

2017-12-01

The Naval Research Laboratory is developing an Earth System Model (NESM) to provide global environmental information to meet Navy and Department of Defense (DoD) operations and planning needs from the upper atmosphere to under the sea. This system consists of a global atmosphere, ocean, ice, wave, and land prediction models and the individual models include: atmosphere - NAVy Global Environmental Model (NAVGEM); ocean - HYbrid Coordinate Ocean Model (HYCOM); sea ice - Community Ice CodE (CICE); WAVEWATCH III™; and land - NAVGEM Land Surface Model (LSM). Data assimilation is currently loosely coupled between the atmosphere component using a 6-hour update cycle in the Naval Research Laboratory (NRL) Atmospheric Variational Data Assimilation System - Accelerated Representer (NAVDAS-AR) and the ocean/ice components using a 24-hour update cycle in the Navy Coupled Ocean Data Assimilation (NCODA) with 3 hours of incremental updating. This presentation will describe the US Navy's coupled forecast model, the loosely coupled data assimilation, and compare results against stand-alone atmosphere and ocean/ice models. In particular, we will focus on the unique aspects of this modeling system, which includes an eddy resolving ocean model and challenges associated with different update-windows and solvers for the data assimilation in the atmosphere and ocean. Results will focus on typical operational diagnostics for atmosphere, ocean, and ice analyses including 500 hPa atmospheric height anomalies, low-level winds, temperature/salinity ocean depth profiles, ocean acoustical proxies, sea ice edge, and sea ice drift. Overall, the global coupled system is performing with comparable skill to the stand-alone systems.

SURFEX v8.0 interface with OASIS3-MCT to couple atmosphere with hydrology, ocean, waves and sea-ice models, from coastal to global scales

NASA Astrophysics Data System (ADS)

Voldoire, Aurore; Decharme, Bertrand; Pianezze, Joris; Lebeaupin Brossier, Cindy; Sevault, Florence; Seyfried, Léo; Garnier, Valérie; Bielli, Soline; Valcke, Sophie; Alias, Antoinette; Accensi, Mickael; Ardhuin, Fabrice; Bouin, Marie-Noëlle; Ducrocq, Véronique; Faroux, Stéphanie; Giordani, Hervé; Léger, Fabien; Marsaleix, Patrick; Rainaud, Romain; Redelsperger, Jean-Luc; Richard, Evelyne; Riette, Sébastien

2017-11-01

This study presents the principles of the new coupling interface based on the SURFEX multi-surface model and the OASIS3-MCT coupler. As SURFEX can be plugged into several atmospheric models, it can be used in a wide range of applications, from global and regional coupled climate systems to high-resolution numerical weather prediction systems or very fine-scale models dedicated to process studies. The objective of this development is to build and share a common structure for the atmosphere-surface coupling of all these applications, involving on the one hand atmospheric models and on the other hand ocean, ice, hydrology, and wave models. The numerical and physical principles of SURFEX interface between the different component models are described, and the different coupled systems in which the SURFEX OASIS3-MCT-based coupling interface is already implemented are presented.

Source term estimation of radioxenon released from the Fukushima Dai-ichi nuclear reactors using measured air concentrations and atmospheric transport modeling.

PubMed

Eslinger, P W; Biegalski, S R; Bowyer, T W; Cooper, M W; Haas, D A; Hayes, J C; Hoffman, I; Korpach, E; Yi, J; Miley, H S; Rishel, J P; Ungar, K; White, B; Woods, V T

2014-01-01

Systems designed to monitor airborne radionuclides released from underground nuclear explosions detected radioactive fallout across the northern hemisphere resulting from the Fukushima Dai-ichi Nuclear Power Plant accident in March 2011. Sampling data from multiple International Modeling System locations are combined with atmospheric transport modeling to estimate the magnitude and time sequence of releases of (133)Xe. Modeled dilution factors at five different detection locations were combined with 57 atmospheric concentration measurements of (133)Xe taken from March 18 to March 23 to estimate the source term. This analysis suggests that 92% of the 1.24 × 10(19) Bq of (133)Xe present in the three operating reactors at the time of the earthquake was released to the atmosphere over a 3 d period. An uncertainty analysis bounds the release estimates to 54-129% of available (133)Xe inventory. Copyright © 2013 Elsevier Ltd. All rights reserved.

Coupled Human-Atmosphere-System Thinking

NASA Astrophysics Data System (ADS)

Schmale, Julia; Chabay, Ilan

2014-05-01

With the discovery of fire, humankind started changing the composition of the atmosphere. Beginning with the industrial revolution, this has led to significant environmental problems, mainly air pollution and climate change. While climate change has been recognized as one key challenge of the Anthropocene, air pollution contributes to the top causes of global premature mortality. Air pollution also plays a key role in contamination of ecosystems and bio-magnification of toxins along food chains. Even though emissions leading to air pollution and climate change often originate from the same sources, they are generally perceived and regulated separately. Climate change impacts are global and hence are tackled at an international level. Conversely, air pollution has local to regional impacts and is thus a matter of national or regional legislation. This legislative and policy divide is generally useful, since full integration could lead, for example, to detrimental delays in action against air pollution through protracted international climate negotiations. However, the separation obscures the fact that almost any kind of human activity leads to the simultaneous emission of air pollutants, toxins and long-lived greenhouse gases. The atmosphere functions as a "dump" for human generated gaseous waste, which is then dispersed and transformed, partly chemically and partly micro-physically, perturbing natural processes in the atmosphere and leading to manifold impacts. In addition, air pollutants affect the Earth's radiative balance directly and indirectly, hence affecting climate change, while a changing climate in turn affects air pollution. Current policies often neglect these linkages and favor mitigation in one arena, which sometimes has detrimental effects on the other. One example is domestic wood burning, which though nearly carbon neutral, deteriorates air quality. Moreover, the design of appliances, machinery, or infrastructure generally does not attempt to minimize atmospheric release, but rather only complies with either climate or air quality requirements. Nor do current narratives promote behavioral change for the overall reduction of emissions (e.g., you can drive your diesel SUV as long as it has a low fuel consumption). This divide and thinking has not only been manifested in policy and regulations and hence media coverage, but has also shaped the public's general perception of this issue. There is no public conceptual understanding regarding humanity's modification of the atmosphere through the continuously and simultaneously released substances by almost any kind of activity and resulting impacts. Here, we propose a conceptual framework that provides a new perspective on the coupled human-atmosphere-system. It makes tangible the inherent linkages between the socio-economic system, the atmospheric physico-chemical changes and impacts, and legal frameworks for sustainable transformations at all levels. To implement HAS-thinking in decision and policy making, both salient disciplinary and interdisciplinary research and comprehensive science-society interactions in the form of transdisciplinary research are necessary. Societal transformations for the sake of a healthy human-atmosphere relationship are highly context dependent and require discussions of normative and value-related issues, which can only be solved through co-designed solutions. We demonstrate the importance of HAS-thinking by examples of sustainable development in the Arctic and Himalayan countries.

An assessment on the environmental contamination caused by the Fukushima accident.

PubMed

Song, Jin Ho

2018-01-15

The radiological releases from the damaged fuel to the atmosphere and into the cooling water in the Fukushima Daiich Nuclear Power Plant (FDNPP) accident are investigated. Atmospheric releases to the land and ocean mostly occurred during the first week after the accident whereas continuous release from the damaged fuel into the cooling water resulted in an accumulation of contaminated water in the plant during last six years. An evaluation of measurement data and analytical model for the release of radionuclides indicated that atmospheric releases were mainly governed by the volatility of the radionuclides. Using the measurement data on the contaminated water, the mechanism for the release of long-lived radionuclides into the cooling water was analyzed. It was found that the radioactivity concentrations of 90 Sr in the contaminated water in the Primary Containment Vessel (PCV) of unit 2 and unit 3 were consistently higher than that of 137 Cs and the radioactivity concentration of 90 Sr in the turbine building of unit 1 in year 2015 was higher than that in year 2011. It was also observed that the radioactivity concentration of long-lived radionuclides in the contaminated water in the FDNPP is still high even in year 2015. The activity ratio of 238 Pu/ 239+240 Pu for the contaminated water was in the range of 1.7-5.4, which was significantly different from the ratios from the soil samples representing the atmospheric releases of FDNPP. It is concluded that the release mechanisms into the atmosphere and cooling water are clearly different and there has been significant amount of long-lived radionuclides released into the contaminated water. Copyright © 2017 Elsevier Ltd. All rights reserved.

Source Term Estimation of Radioxenon Released from the Fukushima Dai-ichi Nuclear Reactors Using Measured Air Concentrations and Atmospheric Transport Modeling

DOE Office of Scientific and Technical Information (OSTI.GOV)

Eslinger, Paul W.; Biegalski, S.; Bowyer, Ted W.

2014-01-01

Systems designed to monitor airborne radionuclides released from underground nuclear explosions detected radioactive fallout from the Fukushima Daiichi nuclear accident in March 2011. Atmospheric transport modeling (ATM) of plumes of noble gases and particulates were performed soon after the accident to determine plausible detection locations of any radioactive releases to the atmosphere. We combine sampling data from multiple International Modeling System (IMS) locations in a new way to estimate the magnitude and time sequence of the releases. Dilution factors from the modeled plume at five different detection locations were combined with 57 atmospheric concentration measurements of 133-Xe taken from Marchmore » 18 to March 23 to estimate the source term. This approach estimates that 59% of the 1.24×1019 Bq of 133-Xe present in the reactors at the time of the earthquake was released to the atmosphere over a three day period. Source term estimates from combinations of detection sites have lower spread than estimates based on measurements at single detection sites. Sensitivity cases based on data from four or more detection locations bound the source term between 35% and 255% of available xenon inventory.« less

Influence of coupling on atmosphere, sea ice and ocean regional models in the Ross Sea sector, Antarctica

NASA Astrophysics Data System (ADS)

Jourdain, Nicolas C.; Mathiot, Pierre; Gallée, Hubert; Barnier, Bernard

2011-04-01

Air-sea ice-ocean interactions in the Ross Sea sector form dense waters that feed the global thermohaline circulation. In this paper, we develop the new limited-area ocean-sea ice-atmosphere coupled model TANGO to simulate the Ross Sea sector. TANGO is built up by coupling the atmospheric limited-area model MAR to a regional configuration of the ocean-sea ice model NEMO. A method is then developed to identify the mechanisms by which local coupling affects the simulations. TANGO is shown to simulate realistic sea ice properties and atmospheric surface temperatures. These skills are mostly related to the skills of the stand alone atmospheric and oceanic models used to build TANGO. Nonetheless, air temperatures over ocean and winter sea ice thickness are found to be slightly improved in coupled simulations as compared to standard stand alone ones. Local atmosphere ocean feedbacks over the open ocean are found to significantly influence ocean temperature and salinity. In a stand alone ocean configuration, the dry and cold air produces an ocean cooling through sensible and latent heat loss. In a coupled configuration, the atmosphere is in turn moistened and warmed by the ocean; sensible and latent heat loss is therefore reduced as compared to the stand alone simulations. The atmosphere is found to be less sensitive to local feedbacks than the ocean. Effects of local feedbacks are increased in the coastal area because of the presence of sea ice. It is suggested that slow heat conduction within sea ice could amplify the feedbacks. These local feedbacks result in less sea ice production in polynyas in coupled mode, with a subsequent reduction in deep water formation.

Synchronizing Two AGCMs via Ocean-Atmosphere Coupling (Invited)

NASA Astrophysics Data System (ADS)

Kirtman, B. P.

2009-12-01

A new approach for fusing or synchronizing to very different Atmospheric General Circulation Models (AGCMs) is described. The approach is also well suited for understand why two different coupled models have such large differences in their respective climate simulations. In the application presented here, the differences between the coupled models using the Center for Ocean-Land-Atmosphere Studies (COLA) and the National Center for Atmospheric Research (NCAR) atmospheric general circulation models (AGCMs) are examined. The intent is to isolate which component of the air-sea fluxes is most responsible for the differences between the coupled models and for the errors in their respective coupled simulations. The procedure is to simultaneously couple the two different atmospheric component models to a single ocean general circulation model (OGCM), in this case the Modular Ocean Model (MOM) developed at the Geophysical Fluid Dynamics Laboratory (GFDL). Each atmospheric component model experiences the same SST produced by the OGCM, but the OGCM is simultaneously coupled to both AGCMs using a cross coupling strategy. In the first experiment, the OGCM is coupled to the heat and fresh water flux from the NCAR AGCM (Community Atmospheric Model; CAM) and the momentum flux from the COLA AGCM. Both AGCMs feel the same SST. In the second experiment, the OGCM is coupled to the heat and fresh water flux from the COLA AGCM and the momentum flux from the CAM AGCM. Again, both atmospheric component models experience the same SST. By comparing these two experimental simulations with control simulations where only one AGCM is used, it is possible to argue which of the flux components are most responsible for the differences in the simulations and their respective errors. Based on these sensitivity experiments we conclude that the tropical ocean warm bias in the COLA coupled model is due to errors in the heat flux, and that the erroneous westward shift in the tropical Pacific cold tongue minimum in the NCAR model is due errors in the momentum flux. All the coupled simulations presented here have warm biases along the eastern boundary of the tropical oceans suggesting that the problem is common to both AGCMs. In terms of interannual variability in the tropical Pacific, the CAM momentum flux is responsible for the erroneous westward extension of the sea surface temperature anomalies (SSTA) and errors in the COLA momentum flux cause the erroneous eastward migration of the El Niño-Southern Oscillation (ENSO) events. These conclusions depend on assuming that the error due to the OGCM can be neglected.

Analysis of Radionuclide Releases from the Fukushima Dai-ichi Nuclear Power Plant Accident Part II

NASA Astrophysics Data System (ADS)

Achim, Pascal; Monfort, Marguerite; Le Petit, Gilbert; Gross, Philippe; Douysset, Guilhem; Taffary, Thomas; Blanchard, Xavier; Moulin, Christophe

2014-03-01

The present part of the publication (Part II) deals with long range dispersion of radionuclides emitted into the atmosphere during the Fukushima Dai-ichi accident that occurred after the March 11, 2011 tsunami. The first part (Part I) is dedicated to the accident features relying on radionuclide detections performed by monitoring stations of the Comprehensive Nuclear Test Ban Treaty Organization network. In this study, the emissions of the three fission products Cs-137, I-131 and Xe-133 are investigated. Regarding Xe-133, the total release is estimated to be of the order of 6 × 1018 Bq emitted during the explosions of units 1, 2 and 3. The total source term estimated gives a fraction of core inventory of about 8 × 1018 Bq at the time of reactors shutdown. This result suggests that at least 80 % of the core inventory has been released into the atmosphere and indicates a broad meltdown of reactor cores. Total atmospheric releases of Cs-137 and I-131 aerosols are estimated to be 1016 and 1017 Bq, respectively. By neglecting gas/particulate conversion phenomena, the total release of I-131 (gas + aerosol) could be estimated to be 4 × 1017 Bq. Atmospheric transport simulations suggest that the main air emissions have occurred during the events of March 14, 2011 (UTC) and that no major release occurred after March 23. The radioactivity emitted into the atmosphere could represent 10 % of the Chernobyl accident releases for I-131 and Cs-137.

Soil Moisture-Atmosphere Feedbacks on Atmospheric Tracers: The Effects of Soil Moisture on Precipitation and Near-Surface Chemistry

NASA Astrophysics Data System (ADS)

Tawfik, Ahmed B.

The atmospheric component is described by rapid fluctuations in typical state variables, such as temperature and water vapor, on timescales of hours to days and the land component evolves on daily to yearly timescales. This dissertation examines the connection between soil moisture and atmospheric tracers under varying degrees of soil moisture-atmosphere coupling. Land-atmosphere coupling is defined over the United States using a regional climate model. A newly examined soil moisture-precipitation feedback is identified for winter months extending the previous summer feedback to colder temperature climates. This feedback is driven by the freezing and thawing of soil moisture, leading to coupled land-atmosphere conditions near the freezing line. Soil moisture can also affect the composition of the troposphere through modifying biogenic emissions of isoprene (C5H8). A novel first-order Taylor series decomposition indicates that isoprene emissions are jointly driven by temperature and soil moisture in models. These compounds are important precursors for ozone formation, an air pollutant and a short-lived forcing agent for climate. A mechanistic description of commonly observed relationships between ground-level ozone and meteorology is presented using the concept of soil moisture-temperature coupling regimes. The extent of surface drying was found to be a better predictor of ozone concentrations than temperature or humidity for the Eastern U.S. This relationship is evaluated in a coupled regional chemistry-climate model under several land-atmosphere coupling and isoprene emissions cases. The coupled chemistry-climate model can reproduce the observed soil moisture-temperature coupling pattern, yet modeled ozone is insensitive to changes in meteorology due to the balance between isoprene and the primary atmospheric oxidant, the hydroxyl radical (OH). Overall, this work highlights the importance of soil moisture-atmosphere coupling for previously neglected cold climate regimes, controlling isoprene emissions variability, and providing a processed-based description of observed ozone-meteorology relationships. From the perspective of ozone air quality, the lack of sensitivity of ozone to meteorology suggests a systematic deficiency in chemistry models in high isoprene emission regions. This shortcoming must be addressed to better estimate tropospheric ozone radiative forcing and to understanding how ozone air quality may respond to future warming.

Mercury Abundances and Isotopic Compositions in the Murchison (CM) and Allende (CV)Carbonaceous Chondrites

NASA Technical Reports Server (NTRS)

Lauretta, D. S.; Klaue, B.; Blum, J. D.; Buseck, P. R.

2001-01-01

The abundance and isotopic composition of Hg was determined in bulk samples of both the Murchison (CM) and Allende (CV) carbonaceous chondrites using single- and multi-collector inductively coupled plasma mass spectrometry (ICP-MS). The bulk abundances of Hg are 294 6 15 ng/g in Murchison and 30.0 6 1.5 ng/g in Allende. These values are within the range of previous measurements of bulk Hg abundances by neutron activation analysis (NAA). Prior studies suggested that both meteorites contain isotopically anomalous Hg, with d l 96/202Hg values for the anomalous, thermal-release components from bulk samples ranging from 2260 %o to 1440 9/00 in Murchison and from 2620 9/00 to 1540 9/00 in Allende (Jovanovic and Reed, 1976a; 1976b; Kumar and Goel, 1992). Our multi-collector ICP-MS measurements suggest that the relative abundances of all seven stable Hg isotopes in both meteorites are identical to terrestrial values within 0.2 to 0.5 9/00m. On-line thermal-release experiments were performed by coupling a programmable oven with the singlecollector ICP-MS. Powdered aliquots of each meteorite were linearly heated from room temperature to 900 C over twenty-five minutes under an Ar atmosphere to measure the isotopic composition of Hg released fiom the meteorites as a h c t i o n of temperature. In separate experiments, the release profiles of S and Se were determined simultaneously with Hg to constrain the Hg distribution within the meteorites and to evaluate the possibility of Se interferences in previous NAA studies. The Hg-release patterns differ between Allende and Murchison. The Hg-release profile for Allende contains two distinct peaks, at 225" and 343"C, whereas the profile for Murchison has only one peak, at 344 C. No isotopically anomalous Hg was detected in the thermal-release experiments at a precision level of 5 to 30 9/00, depending on the isotope ratio. In both meteorites the Hg peak at ;340"C correlates with a peak in the S-release profile. This correlation suggests that Hg is associated with S-bearing phases and, thus, that HgS is a major Hg-bearing phase in both meteorites. The Hg peak at 225 C for Allende is similar to release patterns of physically adsorbed Hg on silicate and metal grains.

Atmosphere-Wave-Ocean Coupling from Regional to Global Earth System Models for High-Impact Extreme Weather Prediction

NASA Astrophysics Data System (ADS)

Chen, S. S.; Curcic, M.

2017-12-01

The need for acurrate and integrated impact forecasts of extreme wind, rain, waves, and storm surge is growing as coastal population and built environment expand worldwide. A key limiting factor in forecasting impacts of extreme weather events associated with tropical cycle and winter storms is fully coupled atmosphere-wave-ocean model interface with explicit momentum and energy exchange. It is not only critical for accurate prediction of storm intensity, but also provides coherent wind, rian, ocean waves and currents forecasts for forcing for storm surge. The Unified Wave INterface (UWIN) has been developed for coupling of the atmosphere-wave-ocean models. UWIN couples the atmosphere, wave, and ocean models using the Earth System Modeling Framework (ESMF). It is a physically based and computationally efficient coupling sytem that is flexible to use in a multi-model system and portable for transition to the next generation global Earth system prediction mdoels. This standardized coupling framework allows researchers to develop and test air-sea coupling parameterizations and coupled data assimilation, and to better facilitate research-to-operation activities. It has been used and extensively tested and verified in regional coupled model forecasts of tropical cycles and winter storms (Chen and Curcic 2016, Curcic et al. 2016, and Judt et al. 2016). We will present 1) an overview of UWIN and its applications in fully coupled atmosphere-wave-ocean model predictions of hurricanes and coastal winter storms, and 2) implenmentation of UWIN in the NASA GMAO GEOS-5.

Acquisition and Early Losses of Rare Gases from the Deep Earth

NASA Technical Reports Server (NTRS)

Porcelli, D.; Cassen, P.; Woolum, D.; Wasserburg, G. J.

1998-01-01

Direct observations show that the deep Earth contains rare gases of solar composition distinct from those in the atmosphere. We examine the implications of mantle rare gas characteristics on acquisition of rare gases from the solar nebula and subsequent losses due to a large impact. Deep mantle rare gas concentrations and isotopic compositions can be obtained from a model of transport and distribution of mantle rare gases. This model assumes the lower mantle closed early, while the upper mantle is open to subduction from the atmosphere and mass transfer from the lower mantle. Constraints are derived that can be incorporated into models for terrestrial volatile acquisition: (1) Calculated lower-mantle Xe-isotopic ratios indicate that the fraction of radiogenic Xe produced by I-129 and Pu-244 during the first about 10(exp 8) yr was lost, a conclusion also drawn for atmospheric Xe. Thus, either the Earth was made from materials that had lost >99% of rare gases about (0.7-2) x 10(exp 8) yr after the solar system formed, or gases were then lost from the fully formed Earth. (2) Concentrations of 3He and 20Ne in the lower mantle were established after these losses. (3) Neon-isotopic data indicates that mantle Ne has solar composition. The model allows for solar Ar/Ne and Xe/Ne in the lower mantle if a dominant fraction of upper mantle Ar and Xe are subduction-derived. If Earth formed in the presence of the solar nebula, it could have been melted by accretional energy and the blanketing effect of a massive, nebula-derived atmosphere. Gases from this atmosphere would have been sequestered within the molten Earth by dissolution at the surface and downward mixing. It was found that too much Ne would be dissolved in the Earth unless the atmosphere began to escape when the Earth was only partially assembled. Here we consider conditions required to initially dissolve sufficient rare gases to account for the present lower mantle concentrations after subsequent losses at 10(exp 8) yr. It is assumed that equilibration of the atmosphere with a thoroughly molten mantle was rapid, so that initial abundances of gases retained in any mantle layer reflected surface conditions when the layer solidified. For subsequent gas loss of 99.5% and typical solubility coefficients, a total pressure of 100 atm was required for an atmosphere of solar composition. Calculations of the pressure at the base of a primordial atmosphere indicate that this value might be exceeded by an order of magnitude or more for an atmosphere supported by accretional energy. Surface temperatures of about 4000 K would have been produced, probably high enough to melt the deep mantle. Initial distributions of retained rare gases would then be determined by the history of surface pressure and temperature during mantle cooling and solidification, i.e., the coupled cooling of Earth and atmosphere. The Earth's thermal state was determined by its surface temperature and the efficiency of convection in the molten mantle, estimated to be sufficient to maintain an adiabatic gradient. Because the melting curve is steeper than the adiabat, solidification of the mantle proceeded outward from the interior. Incorporation of atmospheric gases in the mantle therefore occurred over a range in surface temperature of a few thousand degrees Kelvin. The thermal state of the atmosphere was controlled by total luminosity of the Earth (energy) released by accreting planetesimals and the cooling Earth), nebular temperature and pressure, and atmospheric opacity. The energy released by accretion declined with time as did nebular pressure. Analytical solutions for an idealized (constant opacity radiative atmosphere show that declining energy sources under constant nebular conditions result in slowly diminishing surface temperature but dramatically increasing surface pressure. For such an atmosphere with declining nebular pressure but constant total luminosity, surface pressure decreases gradually with decreasing temperaure. A decline in accretion luminosity might be compensated by energy released as the mantle cools for about 10(exp 5) year, after which luminosity must decline. The total complement of dissolved rare gases will depend on the particular evolutionary path determined by the declining accretional luminosity, the Earth thermal history, removal of the nebula, and opacity variations of the atmosphere. Models for these coupled evolutionary histories for Earth's acquisition of nebular-derived noble gases are in progress. The later losses required at about 10(exp 8) yr (depleting the interior concentrations of the sequestered solar gases by a factor of > 100) were presumably related to the major impact in which the Moon formed.

Coupling tree rings and eddy covariance to estimate long-term above and belowground carbon storage at the stand level

NASA Astrophysics Data System (ADS)

Dye, A.; Alexander, M. R.; Bishop, D.; Pederson, N.; Hessl, A. E.

2016-12-01

Storage of carbon in terrestrial plants and soils directly reduces atmospheric carbon concentration, and it is thereby imperative to improve our understanding of where carbon is being stored and released in an ecosystem and how storages and releases are changing over time. At data-rich sites, coupling alternative measurements of carbon flux can improve this understanding. Here, we present a methodology to inversely model stand-level net storage and release of above- and belowground carbon over a period of 1-2 decades using co-located tree-ring plots and eddy covariance towers at three eastern U.S. forests. We reconstructed annual aboveground wood production (aNPP) from tree rings collected near eddy covariance towers. We compared our aNPP reconstructions with annual tower NEE to address whether interannual variations are correlated. Despite modest correlation, we observed magnitude differences between both records that vary annually. We interpret these differences as indicative of changes in belowground carbon storage, i.e. an aNPP:NEE ratio > 1 indicates a net release of belowground carbon and a ratio < 1 a net storage of belowground carbon. For this interpretation, we assume the following: a) carbon not directed to above or belowground pools is insignificant, b) carbon not stored above ground is stored below ground, and c) mature trees do not add to a storage pool at a higher level every year. While the offset between biometric aNPP and tower NEE could partially be attributed to the diversion of assimilated carbon to nonstructural carbohydrates instead of growth, we argue that this becomes a less important factor over longer time scales in a mature tree. Our approach does not quantify belowground NPP or allocation, but we present a method for estimating belowground carbon storage and release at the stand level, an otherwise difficult task at this scale due to heterogeneity across the stand.

A physics-based model for the ionization of samarium by the MOSC chemical releases in the upper atmosphere

NASA Astrophysics Data System (ADS)

Bernhardt, Paul A.; Siefring, Carl L.; Briczinski, Stanley J.; Viggiano, Albert; Caton, Ronald G.; Pedersen, Todd R.; Holmes, Jeffrey M.; Ard, Shaun; Shuman, Nicholas; Groves, Keith M.

2017-05-01

Atomic samarium has been injected into the neutral atmosphere for production of electron clouds that modify the ionosphere. These electron clouds may be used as high-frequency radio wave reflectors or for control of the electrodynamics of the F region. A self-consistent model for the photochemical reactions of Samarium vapor cloud released into the upper atmosphere has been developed and compared with the Metal Oxide Space Cloud (MOSC) experimental observations. The release initially produces a dense plasma cloud that that is rapidly reduced by dissociative recombination and diffusive expansion. The spectral emissions from the release cover the ultraviolet to the near infrared band with contributions from solar fluorescence of the atomic, molecular, and ionized components of the artificial density cloud. Barium releases in sunlight are more efficient than Samarium releases in sunlight for production of dense ionization clouds. Samarium may be of interest for nighttime releases but the artificial electron cloud is limited by recombination with the samarium oxide ion.

Local atmospheric response to warm mesoscale ocean eddies in the Kuroshio-Oyashio Confluence region.

PubMed

Sugimoto, Shusaku; Aono, Kenji; Fukui, Shin

2017-09-19

In the extratropical regions, surface winds enhance upward heat release from the ocean to atmosphere, resulting in cold surface ocean: surface ocean temperature is negatively correlated with upward heat flux. However, in the western boundary currents and eddy-rich regions, the warmer surface waters compared to surrounding waters enhance upward heat release-a positive correlation between upward heat release and surface ocean temperature, implying that the ocean drives the atmosphere. The atmospheric response to warm mesoscale ocean eddies with a horizontal extent of a few hundred kilometers remains unclear because of a lack of observations. By conducting regional atmospheric model experiments, we show that, in the Kuroshio-Oyashio Confluence region, wintertime warm eddies heat the marine atmospheric boundary layer (MABL), and accelerate westerly winds in the near-surface atmosphere via the vertical mixing effect, leading to wind convergence around the eastern edge of eddies. The warm-eddy-induced convergence forms local ascending motion where convective precipitation is enhanced, providing diabatic heating to the atmosphere above MABL. Our results indicate that warm eddies affect not only near-surface atmosphere but also free atmosphere, and possibly synoptic atmospheric variability. A detailed understanding of warm eddy-atmosphere interaction is necessary to improve in weather and climate projections.

Recharge of the early atmosphere of Mars by impact-induced release of CO2

USGS Publications Warehouse

Carr, Michael H.

1989-01-01

Channels on the Martian surface suggest that Mars had an early, relatively thick atmosphere. If the atmosphere was thick enough for water to be stable at the surface, CO2 in the atmosphere would have been fixed as carbonates on a relatively short time scale, previously estimated to be 1 bar every 107 years. This loss must have been offset by some replenishment mechanism to account for the numerous valley networks in the oldest surviving terrains. Impacts could have released CO2 into the atmosphere by burial, by shock-induced release during impact events, and by addition of carbon to Mars from the impacting bolides. Depending on the relationship between the transient cavity diameter and the diameter of the resulting crater, burial rates as a result of impact gardening at the end of heavy bombardment are estimated to range from 20 to 45 m/106 years, on the assumption that cratering rates in Mars were similar to those of the Nectarian Period on the Moon. At these rates 0.1-0.2 bar of CO2 could have been released every 107 years as a result of burial to depths where dissociation temperatures of carbonates were reached. Modeling of large impacts suggests that an additional 0.01 to 0.02 bar of CO2 could have been released every 107 years during the actual impacts. In the unlikely event that all the impacting material was composed of carbonaceous chondrites, a further 0.3 bar of CO2 could have been added to the atmosphere every 107 years by oxidation of meteoritic carbon. Even when supplemented by the volcanically induced release of CO2, these release rates are barely sufficient to sustain an early atmosphere if water were continuously present at the surface. The results suggest that water may have been only intermittently present on the surface early in the planet's history.

Probabilistic safety analysis for urgent situations following the accidental release of a pollutant in the atmosphere

NASA Astrophysics Data System (ADS)

Armand, P.; Brocheton, F.; Poulet, D.; Vendel, F.; Dubourg, V.; Yalamas, T.

2014-10-01

This paper is an original contribution to uncertainty quantification in atmospheric transport & dispersion (AT&D) at the local scale (1-10 km). It is proposed to account for the imprecise knowledge of the meteorological and release conditions in the case of an accidental hazardous atmospheric emission. The aim is to produce probabilistic risk maps instead of a deterministic toxic load map in order to help the stakeholders making their decisions. Due to the urge attached to such situations, the proposed methodology is able to produce such maps in a limited amount of time. It resorts to a Lagrangian particle dispersion model (LPDM) using wind fields interpolated from a pre-established database that collects the results from a computational fluid dynamics (CFD) model. This enables a decoupling of the CFD simulations from the dispersion analysis, thus a considerable saving of computational time. In order to make the Monte-Carlo-sampling-based estimation of the probability field even faster, it is also proposed to recourse to the use of a vector Gaussian process surrogate model together with high performance computing (HPC) resources. The Gaussian process (GP) surrogate modelling technique is coupled with a probabilistic principal component analysis (PCA) for reducing the number of GP predictors to fit, store and predict. The design of experiments (DOE) from which the surrogate model is built, is run over a cluster of PCs for making the total production time as short as possible. The use of GP predictors is validated by comparing the results produced by this technique with those obtained by crude Monte Carlo sampling.

Thermal characterization of Titan's tholins by simultaneous TG-MS, DTA, DSC analysis

NASA Astrophysics Data System (ADS)

Nna-Mvondo, Delphine; de la Fuente, José L.; Ruiz-Bermejo, Marta; Khare, Bishun; McKay, Christopher P.

2013-09-01

Three samples of Titan's tholins synthesized in laboratory under simulated Titan's conditions and presenting different degrees of exposure to ambient atmosphere have been used to study in detail their thermal behavior using thermogravimetry coupled with a mass spectrometer (TG-MS), differential thermal analysis (DTA) and differential scanning calorimetry (DSC). The degradation of Titan's tholins under inert atmosphere follows a three-step consecutive decomposition: a drying stage (>150 °C) where moisture is desorbed, this stage indicated the high hydrophilicity of the tholins; a second stage, the main pyrolysis stage (150-575 °C) where endothermic decomposition begins releasing mainly ammonia, HCN, acetonitrile, and methane over a broad temperature range. Few other hydrocarbon fragments such as ethylene and propane are released but no cyclic molecules, aliphatic or aromatic, are observed. The last stage (>575 °C) is the carbonization of the material leading to a non-crystalline graphitic residue. The thermal degradation under oxygen atmosphere shows the same stages as in argon, with a shift of the thermogravimetric peaks toward lower temperatures indicating a lower thermal stability. The last stage in this case is an oxidative combustion of the char residue. This research concludes that even if Titan tholins, subjected to air contamination for few minutes to several years (varying with the storage conditions) transform to produce different C/N and C/O ratios and thermal stabilities, they undergo the same thermal degradation phases and products. This suggests that the studied three tholins have a similar main chemical structure which does not alter by the air exposure. We discuss on the possible nature of this structure.

Fiber-coupling efficiency for free-space optical communication through atmospheric turbulence.

PubMed

Dikmelik, Yamaç; Davidson, Frederic M

2005-08-10

High-speed free-space optical communication systems have recently used fiber-optic components. The received laser beam in such a system must be coupled into a single-mode fiber at the input of the receiver module. However, propagation through atmospheric turbulence degrades the spatial coherence of a laser beam and limits the fiber-coupling efficiency. We numerically evaluate the fiber-coupling efficiency for laser light distorted by atmospheric turbulence. We also investigate the use of a coherent fiber array as a receiver structure and find that a coherent fiber array that consists of seven subapertures would significantly increase the fiber-coupling efficiency.

Atmospheric propagation modeling indicates homing pigeons use loft-specific infrasonic 'map' cues.

PubMed

Hagstrum, Jonathan T

2013-02-15

Results from an acoustic ray-tracing program using daily meteorological profiles are presented to explain 'release-site biases' for homing pigeons at three experimental sites in upstate New York where W. T. Keeton and his co-workers at Cornell University conducted extensive releases between 1968 and 1987 in their investigations of the avian navigational 'map'. The sites are the Jersey Hill and Castor Hill fire towers, and another near Weedsport, where control pigeons from the Cornell loft vanished in random directions, in directions consistently >50 deg clockwise and in directions ∼15 deg clockwise from the homeward bearing, respectively. Because Cornell pigeons were disoriented at Jersey Hill whereas birds from other lofts were not, it is inferred that Jersey Hill lies within an acoustic 'shadow' zone relative to infrasonic signals originating from the Cornell loft's vicinity. Such signals could arise from ground-to-air coupling of near-continuous microseisms, or from scattering of direct microbaroms off terrain features, both of which are initially generated by wave-wave interactions in the deep ocean. HARPA runs show that little or no infrasound from the loft area arrived at Jersey Hill on days when Cornell pigeons were disoriented there, and that homeward infrasonic signals could have arrived at all three sites from directions consistent with pigeon departure bearings, especially on days when these bearings were unusual. The general stability of release-site biases might be due to influences of terrain on transmission of the homeward signals under prevailing weather patterns, whereas short-term changes in biases might be caused by rapid shifts in atmospheric conditions.

Atmospheric propagation modeling indicates homing pigeons use loft-specific infrasonic ‘map’ cues

USGS Publications Warehouse

Hagstrum, Jonathan T.

2013-01-01

Results from an acoustic ray-tracing program using daily meteorological profiles are presented to explain ‘release-site biases’ for homing pigeons at three experimental sites in upstate New York where W. T. Keeton and his co-workers at Cornell University conducted extensive releases between 1968 and 1987 in their investigations of the avian navigational ‘map’. The sites are the Jersey Hill and Castor Hill fire towers, and another near Weedsport, where control pigeons from the Cornell loft vanished in random directions, in directions consistently >50 deg clockwise and in directions ∼15 deg clockwise from the homeward bearing, respectively. Because Cornell pigeons were disoriented at Jersey Hill whereas birds from other lofts were not, it is inferred that Jersey Hill lies within an acoustic ‘shadow’ zone relative to infrasonic signals originating from the Cornell loft’s vicinity. Such signals could arise from ground-to-air coupling of near-continuous microseisms, or from scattering of direct microbaroms off terrain features, both of which are initially generated by wave–wave interactions in the deep ocean. HARPA runs show that little or no infrasound from the loft area arrived at Jersey Hill on days when Cornell pigeons were disoriented there, and that homeward infrasonic signals could have arrived at all three sites from directions consistent with pigeon departure bearings, especially on days when these bearings were unusual. The general stability of release-site biases might be due to influences of terrain on transmission of the homeward signals under prevailing weather patterns, whereas short-term changes in biases might be caused by rapid shifts in atmospheric conditions.

Shifting carbon flow from roots into associated microbial communities in response to elevated atmospheric CO2.

PubMed

Drigo, Barbara; Pijl, Agata S; Duyts, Henk; Kielak, Anna M; Gamper, Hannes A; Houtekamer, Marco J; Boschker, Henricus T S; Bodelier, Paul L E; Whiteley, Andrew S; van Veen, Johannes A; Kowalchuk, George A

2010-06-15

Rising atmospheric CO(2) levels are predicted to have major consequences on carbon cycling and the functioning of terrestrial ecosystems. Increased photosynthetic activity is expected, especially for C-3 plants, thereby influencing vegetation dynamics; however, little is known about the path of fixed carbon into soil-borne communities and resulting feedbacks on ecosystem function. Here, we examine how arbuscular mycorrhizal fungi (AMF) act as a major conduit in the transfer of carbon between plants and soil and how elevated atmospheric CO(2) modulates the belowground translocation pathway of plant-fixed carbon. Shifts in active AMF species under elevated atmospheric CO(2) conditions are coupled to changes within active rhizosphere bacterial and fungal communities. Thus, as opposed to simply increasing the activity of soil-borne microbes through enhanced rhizodeposition, elevated atmospheric CO(2) clearly evokes the emergence of distinct opportunistic plant-associated microbial communities. Analyses involving RNA-based stable isotope probing, neutral/phosphate lipid fatty acids stable isotope probing, community fingerprinting, and real-time PCR allowed us to trace plant-fixed carbon to the affected soil-borne microorganisms. Based on our data, we present a conceptual model in which plant-assimilated carbon is rapidly transferred to AMF, followed by a slower release from AMF to the bacterial and fungal populations well-adapted to the prevailing (myco-)rhizosphere conditions. This model provides a general framework for reappraising carbon-flow paths in soils, facilitating predictions of future interactions between rising atmospheric CO(2) concentrations and terrestrial ecosystems.

Evaluating Carbon and Climate Sensitivities of the NOAA/GFDL Earth System Model ESM2Mb to Forcing Perturbations during the Paleocene-Eocene Thermal Maximum

NASA Astrophysics Data System (ADS)

Tandy, H.; Shevliakova, E.; Keller, G.

2017-12-01

The Paleocene-Eocene Thermal Maximum (PETM, 55.5 Myr) was a period of rapid warming resulting from major changes in the carbon cycle and has been cited as the closest historical analogue to anthropogenic carbon release. Up to now, modeling studies of the PETM used either a low-resolution coupled model of the ocean and atmosphere with prescribed CO2 or CH4, or coupled climate-carbon models of intermediate complexity (i.e. simplified ocean or atmosphere). In this study we carried a suit of numerical experiments with the NOAA/GFDL comprehensive atmosphere-ocean coupled model with integrated terrestrial and marine carbon cycle components, known as an Earth System Model (ESM2Mb). We analyzed the output from millennia-scale ESM2Mb simulations with different combinations of forcings from the pre-PETM and PETM, including greenhouse gas concentrations and solar intensity. In addition we explore sensitivities of climate and carbon cycling to changes in geology such as topography, continental positions, and the presence and absence of large land glaciers. Furthermore, we examine ESM2Mb climate and carbon sensitivities to PETM conditions with a focus on how alternate conditions and forcings relate to the uncertainty in the climate and carbon cycling estimates from paleo observations. We explore changes in atmosphere, land, and ocean temperatures and circulation patterns as well as vegetation distribution, permafrost, and carbon storage in terrestrial and marine ecosystems from pre-PETM to PETM conditions. We found that with the present day land/sea mask and land glaciers in ESM2Mb, changes in only greenhouse gas concentrations (CO2 and CH4) from pre-PETM to PETM conditions induce global warming of 3-5 °C, consistent with the lower range of estimates from paleo proxies. Changes in the carbon permafrost storage from warming cannot explain the rapid increase in the atmospheric CO2 concentration. Changes in the ocean circulation and carbon storage critically depend on geological conditions such as continental positions. The study illustrates how models designed for studying future climate change can capture past paleo events, such as the PETM, and how modern day geological conditions may affect climate and carbon cycle sensitivities.

Impacts of an Ammonia Leak on the Cabin Atmosphere of the International Space Station

NASA Technical Reports Server (NTRS)

Duchesne, Stephanie M.; Sweterlitsch, Jeff J.; Son, Chang H.; Perry, Jay L.

2011-01-01

Toxic chemical release into the cabin atmosphere is one of the three major emergency scenarios identified on the International Space Station (ISS). The release of anhydrous ammonia, the coolant used in the U.S. On-orbit Segment (USOS) External Active Thermal Control Subsystem (EATCS), into the ISS cabin atmosphere is one of the most serious toxic chemical release cases identified on board ISS. The USOS Thermal Control System (TCS) includes an Internal Thermal Control Subsystem (ITCS) water loop and an EATCS ammonia loop that transfer heat at the interface heat exchanger (IFHX). Failure modes exist that could cause a breach within the IFHX. This breach would result in high pressure ammonia from the EATCS flowing into the lower pressure ITCS water loop. As the pressure builds in the ITCS loop, it is likely that the gas trap, which has the lowest maximum design pressure within the ITCS, would burst and cause ammonia to enter the ISS atmosphere. It is crucial to first characterize the release of ammonia into the ISS atmosphere in order to develop methods to properly mitigate the environmental risk. This paper will document the methods used to characterize an ammonia leak into the ISS cabin atmosphere. A mathematical model of the leak was first developed in order to define the flow of ammonia into the ISS cabin atmosphere based on a series of IFHX rupture cases. Computational Fluid Dynamics (CFD) methods were then used to model the dispersion of the ammonia throughout the ISS cabin and determine localized effects and ventilation effects on the dispersion of ammonia. Lastly, the capabilities of the current on-orbit systems to remove ammonia were reviewed and scrubbing rates of the ISS systems were defined based on the ammonia release models. With this full characterization of the release of ammonia from the USOS TCS, an appropriate mitigation strategy that includes crew and system emergency response procedures, personal protection equipment use, and atmosphere monitoring and scrubbing hardware can be established.

Impacts of an Ammonia Leak on the Cabin Atmosphere of the International Space Station

NASA Technical Reports Server (NTRS)

Duchesne, Stephanie M.; Sweterlitsch, Jeffrey J.; Son, Chang H.; Perry Jay L.

2012-01-01

Toxic chemical release into the cabin atmosphere is one of the three major emergency scenarios identified on the International Space Station (ISS). The release of anhydrous ammonia, the coolant used in the U.S. On-orbit Segment (USOS) External Active Thermal Control Subsystem (EATCS), into the ISS cabin atmosphere is one of the most serious toxic chemical release cases identified on board ISS. The USOS Thermal Control System (TCS) includes an Internal Thermal Control Subsystem (ITCS) water loop and an EATCS ammonia loop that transfer heat at the interface heat exchanger (IFHX). Failure modes exist that could cause a breach within the IFHX. This breach would result in high pressure ammonia from the EATCS flowing into the lower pressure ITCS water loop. As the pressure builds in the ITCS loop, it is likely that the gas trap, which has the lowest maximum design pressure within the ITCS, would burst and cause ammonia to enter the ISS atmosphere. It is crucial to first characterize the release of ammonia into the ISS atmosphere in order to develop methods to properly mitigate the environmental risk. This paper will document the methods used to characterize an ammonia leak into the ISS cabin atmosphere. A mathematical model of the leak was first developed in order to define the flow of ammonia into the ISS cabin atmosphere based on a series of IFHX rupture cases. Computational Fluid Dynamics (CFD) methods were then used to model the dispersion of the ammonia throughout the ISS cabin and determine localized effects and ventilation effects on the dispersion of ammonia. Lastly, the capabilities of the current on-orbit systems to remove ammonia were reviewed and scrubbing rates of the ISS systems were defined based on the ammonia release models. With this full characterization of the release of ammonia from the USOS TCS, an appropriate mitigation strategy that includes crew and system emergency response procedures, personal protection equipment use, and atmosphere monitoring and scrubbing hardware can be established.

Evidence of weak land-atmosphere coupling under varying bare soil conditions: Are fully coupled Darcy/Navier-Stokes models necessary for simulating soil moisture dynamics?

NASA Astrophysics Data System (ADS)

Illangasekare, T. H.; Trautz, A. C.; Howington, S. E.; Cihan, A.

2017-12-01

It is a well-established fact that the land and atmosphere form a continuum in which the individual domains are coupled by heat and mass transfer processes such as bare-soil evaporation. Soil moisture dynamics can be simulated at the representative elementary volume (REV) scale using decoupled and fully coupled Darcy/Navier-Stokes models. Decoupled modeling is an asynchronous approach in which flow and transport in the soil and atmosphere is simulated independently; the two domains are coupled out of time-step via prescribed flux parameterizations. Fully coupled modeling in contrast, solves the governing equations for flow and transport in both domains simultaneously with the use of coupling interface boundary conditions. This latter approach, while being able to provide real-time two-dimensional feedbacks, is considerably more complex and computationally intensive. In this study, we investigate whether fully coupled models are necessary, or if the simpler decoupled models can sufficiently capture soil moisture dynamics under varying land preparations. A series of intermediate-scale physical and numerical experiments were conducted in which soil moisture distributions and evaporation estimates were monitored at high spatiotemporal resolutions for different heterogeneous packing and soil roughness scenarios. All experimentation was conducted at the newly developed Center for Experimental Study of Subsurface Environmental Processes (CESEP) wind tunnel-porous media user test-facility at the Colorado School of. Near-surface atmospheric measurements made during the experiments demonstrate that the land-atmosphere coupling was relatively weak and insensitive to the applied edaphic and surface conditions. Simulations with a decoupled multiphase heat and mass transfer model similarly show little sensitivity to local variations in atmospheric forcing; a single, simple flux parameterization can sufficiently capture the soil moisture dynamics (evaporation and redistribution) as long as the subsurface conditions (i.e., heterogeneity) are properly described. These findings suggest that significant improvements to simulations results should not be expected if fully coupled modeling were adopted in scenarios of weak land-atmosphere coupling in the context of bare soil evaporation.

Do we know what difference a delay makes?

NASA Astrophysics Data System (ADS)

Risbey, James S.; Handel, Mark David; Stone, Peter H.

In our original comment [Risbey et al.., 1991] we argued that the work of Schlesinger and Jiang [1991a] is too limited to determine whether or not (as they put it) “the penalty is small for a 10-year delay in initiating the transition to a regime in which greenhouse-gas emissions are reduced.” In their reply, Schlesinger and Jiang [1991b] (hereafter S&J) presented their reasons for concluding definitively that the penalty is small. However S&J's discussion of the evidence and literature on climate change and greenhouse warming contains significant omissions and mis-statements.In dismissing our concern that their model was too simple to evaluate the possibility of abrupt climate change, S&J rely on results from coupled ocean-atmosphere general circulation models (GCMs), in particular the work of Cubasch et al.. [1991]. Here S&J make two claims, one of which is incorrect and the other questionable. First, they claim that “the coupled atmosphere-ocean model of Cubasch et al. [1991] does allow the nonlinearities that Risbey et al.. [1991] criticize our simple model for not including.” In fact we explicitly mentioned changes in polar ice caps [Oerlemans and van der Veen, 1984] and release of methane from clathrates [MacDonald, 1990; Bell, 1982], neither of which are included in the model of Cubasch et al.. [1991]. Indeed, none of the published simulations of global warming using coupled ocean-atmosphere GCMs include these effects. Nor do these models yet include in their enhanced greenhouse simulations many of the possible feedbacks involving the carbon cycle and biosphere [Lashof, 1989; Bacastow and Maier-Reimer, 1990; Sellers, 1987] that could significantly alter greenhouse gas concentrations and surface properties. The published simulations with these models do allow for some changes in deep ocean circulation and cloud behavior, but there is controversy over whether they correctly represent these processes [Marotzke, 1991; Mitchell, 1989; Cess, 1990]. In addition the coupled models must be arbitrarily tuned (requiring substantial artificial fluxes of heat and moisture) to get the current climate right [Manabe et al.., 1991; Cubasch et al.., 1991]. Their greenhouse change simulations are at least partly constrained by these flux adjustments.

Operational coupled atmosphere - ocean - ice forecast system for the Gulf of St. Lawrence, Canada

NASA Astrophysics Data System (ADS)

Faucher, M.; Roy, F.; Desjardins, S.; Fogarty, C.; Pellerin, P.; Ritchie, H.; Denis, B.

2009-09-01

A fully interactive coupled atmosphere-ocean-ice forecasting system for the Gulf of St. Lawrence (GSL) has been running in experimental mode at the Canadian Meteorological Centre (CMC) for the last two winter seasons. The goal of this project is to provide more accurate weather and sea ice forecasts over the GSL and adjacent coastal areas by including atmosphere-oceanice interactions in the CMC operational forecast system using a formal coupling strategy between two independent modeling components. The atmospheric component is the Canadian operational GEM model (Côté et al. 1998) and the oceanic component is the ocean-ice model for the Gulf of St. Lawrence developed at the Maurice Lamontagne Institute (IML) (Saucier et al. 2003, 2004). The coupling between those two models is achieved by exchanging surface fluxes and variables through MPI communication. The re-gridding of the variables is done with a package developed at the Recherche en Prevision Numerique centre (RPN, Canada). Coupled atmosphere - ocean - ice forecasts are issued once a day based on 00GMT data. Results for the past two years have demonstrated that the coupled system produces improved forecasts in and around the GSL during all seasons, proving that atmosphere-ocean-ice interactions are indeed important even for short-term Canadian weather forecasts. This has important implications for other coupled modeling and data assimilation partnerships that are in progress involving EC, the Department of Fisheries and Oceans (DFO) and the National Defense (DND). Following this experimental phase, it is anticipated that this GSL system will be the first fully interactive coupled system to be implemented at CMC.

The influence of cladding on fission gas release from irradiated U-Mo monolithic fuel

NASA Astrophysics Data System (ADS)

Burkes, Douglas E.; Casella, Amanda J.; Casella, Andrew M.

2017-04-01

The monolithic uranium-molybdenum (U-Mo) alloy has been proposed as a fuel design capable of converting the world's highest power research reactors from use of high enriched uranium to low enriched uranium. However, a zirconium (Zr) diffusion barrier must be used to eliminate interactions that form between the U-Mo monolith and aluminum alloy 6061 (AA6061) cladding during fabrication and are enhanced during irradiation. One aspect of fuel development and qualification is to demonstrate an appropriate understanding of the extent of fission product release from the fuel under anticipated service environments. An exothermic reaction has previously been observed between the AA6061 cladding and Zr diffusion layer. In this paper, two fuel segments with different irradiation history were subjected to specified thermal profiles under a controlled atmosphere using a thermogravimetric/differential thermal analyzer coupled with a mass spectrometer inside a hot cell. Samples from each segment were tested with cladding and without cladding to investigate the effect, if any, that the exothermic reaction has on fission gas release mechanisms. Measurements revealed there is an instantaneous effect of the cladding/Zr exothermic reaction, but not necessarily a cumulative effect above approximately 973 K (700 °C). The mechanisms responsible for fission gas release events are discussed.

Amidine-Functionalized Poly(2-vinyl-4,4-dimethylazlactone) for Selective and Efficient CO 2 Fixing

DOE Office of Scientific and Technical Information (OSTI.GOV)

Barkakaty, Balaka; Browning, Katie L.; Sumpter, Bobby

Development of novel polymeric materials capable of efficient CO 2 capture and separation under ambient conditions is crucial for cost-effective and practical industrial applications. Here we report the facile synthesis of a new CO 2-responsive polymer through post-polymerization modification of poly(2 vinyl-4,4-dimethylazlactone) (PVDMA). The reactive pendant azlactone groups of PVDMA are easily modified with 4-(N-methyltetrahydropyrimidine) benzyl alcohol (PBA) without any by-product formation. FTIR and TGA experiments show the new PBA functionalized polymer powder can reversibly capture CO 2 at room temperature and under atmospheric pressure. CO2 capture was selective, showing a high fixing efficiency even with a mixed gas systemmore » (20% CO 2, 80% N 2) similar to flue gas. CO 2 release occurred at room temperature and release profiles were investigated as a function of temperature. Density Functional Theory (DFT) calculations coupled with modeling and simulation reveal the presence of two CO 2 binding sites in the PBA functionalized polymer resulting in a two-step CO 2 release at room temperature. Finally, we find that the ease of material preparation, high fixing efficiency, and robust release characteristics suggest that post-polymerization modification may be a useful route to designing new materials for CO 2 capture.« less

The influence of cladding on fission gas release from irradiated U-Mo monolithic fuel

DOE Office of Scientific and Technical Information (OSTI.GOV)

Burkes, Douglas E.; Casella, Amanda J.; Casella, Andrew M.

2017-04-01

The monolithic uranium-molybdenum (U-Mo) alloy has been proposed as a fuel design capable of converting the world’s highest power research reactors from use of high enriched uranium to low enriched uranium. However, a zirconium (Zr) diffusion barrier must be used to eliminate interactions that form during fabrication and are enhanced during irradiation between the U-Mo monolith and aluminum alloy 6061 (AA6061) cladding. One aspect of fuel development and qualification is to demonstrate appropriate understanding of the extent of fission product release from the fuel under anticipated service environments. An exothermic reaction has previously been observed between the AA6061 cladding andmore » Zr diffusion layer. In this paper, two fuel segments with different irradiation history were subjected to specified thermal profiles under a controlled atmosphere using a thermogravimetric/differential thermal analyzer coupled with a mass spectrometer inside a hot cell. Samples from each segment were tested with cladding and without cladding to investigate the effect, if any, that the exothermic reaction has on fission gas release mechanisms. Measurements revealed there is an instantaneous effect of the cladding/Zr exothermic reaction, but not necessarily a cumulative effect above approximately 973 K (700 oC). The mechanisms responsible for fission gas release events are discussed.« less

Amidine-Functionalized Poly(2-vinyl-4,4-dimethylazlactone) for Selective and Efficient CO 2 Fixing

DOE PAGES

Barkakaty, Balaka; Browning, Katie L.; Sumpter, Bobby; ...

2016-02-12

Development of novel polymeric materials capable of efficient CO 2 capture and separation under ambient conditions is crucial for cost-effective and practical industrial applications. Here we report the facile synthesis of a new CO 2-responsive polymer through post-polymerization modification of poly(2 vinyl-4,4-dimethylazlactone) (PVDMA). The reactive pendant azlactone groups of PVDMA are easily modified with 4-(N-methyltetrahydropyrimidine) benzyl alcohol (PBA) without any by-product formation. FTIR and TGA experiments show the new PBA functionalized polymer powder can reversibly capture CO 2 at room temperature and under atmospheric pressure. CO2 capture was selective, showing a high fixing efficiency even with a mixed gas systemmore » (20% CO 2, 80% N 2) similar to flue gas. CO 2 release occurred at room temperature and release profiles were investigated as a function of temperature. Density Functional Theory (DFT) calculations coupled with modeling and simulation reveal the presence of two CO 2 binding sites in the PBA functionalized polymer resulting in a two-step CO 2 release at room temperature. Finally, we find that the ease of material preparation, high fixing efficiency, and robust release characteristics suggest that post-polymerization modification may be a useful route to designing new materials for CO 2 capture.« less

Medicanes in an ocean-atmosphere coupled regional climate model

NASA Astrophysics Data System (ADS)

Akhtar, Naveed; Brauch, Jennifer; Ahrens, Bodo

2014-05-01

So-called medicanes (Mediterranean hurricanes) are meso-scale, marine and warm core Mediterranean cyclones which exhibit some similarities with tropical cyclones. The strong cyclonic winds associated with them are a potential thread for highly populated coastal areas around the Mediterranean basin. In this study we employ an atmospheric limited-area model (COSMO-CLM) coupled with a one-dimensional ocean model (NEMO-1d) to simulate medicanes. The goal of this study is to assess the robustness of the coupled model to simulate these extreme events. For this purpose 11 historical medicane events are simulated by the atmosphere-only and the coupled models using different set-ups (horizontal grid-spacings: 0.44o, 0.22o, 0.088o; with/with-out spectral nudging). The results show that at high resolution the coupled model is not only able to simulate all medicane events but also improves the simulated track length, warm core, and wind speed of simulated medicanes compared to atmosphere-only simulations. In most of the cases the medicanes trajectories and structures are better represented in coupled simulations compared to atmosphere-only simulations. We conclude that the coupled model is a suitable tool for systemic and detailed study of historical medicane events and also for future projections.

[In vitro release of [5Met]- and [5Leu]-enkephalins from the rat brain crude synaptosomal (P2) fraction: Ca2+-dependency of K+-stimulation and effects of various drugs].

PubMed

Koida, M; Takahashi, M; Takenaga, K

1983-01-01

The rat brain P2 fraction was suspended in Krebs Ringer bicarbonate buffer containing 20 microM bacitracin and incubated at 37 degrees C for 10 min under an atmosphere of 95% O2-5% CO2. Incubation was terminated by centrifugation at 4 degrees C and 10,000 X g for 10 min. The supernatant was designated as the S1 fraction, and from the pellet, the S2 to S4 fractions were collected by repeated suspension, incubation, and centrifugation. The radioimmunoassays of each S fraction revealed the spontaneous release of [5Met]- and [5Leu]-enkephalins at the ratio of 2 to 1. The peptide contents gradually decreased from S1 to S4, but the release tended to become constant in S3 and S4. Thus, the effects of some ions and drugs on the release were compared at the stage of obtaining the S3 fraction. The release of both peptides were significantly stimulated in 50 mM KCl buffer, and the stimulatory effect appears to be dependent on Ca2+ concentration. Veratrine and A23187 were also effective stimulants of the release. On the other hand, neither spontaneous nor K+-stimulated release of enkephalins was affected by morphine (1 microM), naloxone (1 microM), kyotorphin (1 or 10 microM), and Li+ (50 mM). Similar results were obtained with the release of 3H-noradrenaline taken up in vitro by the P2 fraction. The usability of the P2 fraction as an in vitro model for the study of stimulus-coupled release of enkephalins was discussed with some limitations found herein.

Modeling of atmospheric-coupled Rayleigh waves on planets with atmosphere: From Earth observation to Mars and Venus perspectives.

PubMed

Lognonné, Philippe; Karakostas, Foivos; Rolland, Lucie; Nishikawa, Yasuhiro

2016-08-01

Acoustic coupling between solid Earth and atmosphere has been observed since the 1960s, first from ground-based seismic, pressure, and ionospheric sensors and since 20 years with various satellite measurements, including with global positioning system (GPS) satellites. This coupling leads to the excitation of the Rayleigh surface waves by local atmospheric sources such as large natural explosions from volcanoes, meteor atmospheric air-bursts, or artificial explosions. It contributes also in the continuous excitation of Rayleigh waves and associated normal modes by atmospheric winds and pressure fluctuations. The same coupling allows the observation of Rayleigh waves in the thermosphere most of the time through ionospheric monitoring with Doppler sounders or GPS. The authors review briefly in this paper observations made on Earth and describe the general frame of the theory enabling the computation of Rayleigh waves for models of telluric planets with atmosphere. The authors then focus on Mars and Venus and give in both cases the atmospheric properties of the Rayleigh normal modes and associated surface waves compared to Earth. The authors then conclude on the observation perspectives especially for Rayleigh waves excited by atmospheric sources on Mars and for remote ionospheric observations of Rayleigh waves excited by quakes on Venus.

Prolonged Effect of Severe Wildfires on Mercury and Other Volatiles in Forest Soils of the Lake Superior Region, USA

NASA Astrophysics Data System (ADS)

Cannon, W. F.; Woodruff, L. G.

2003-12-01

Soils in Isle Royale National Park, Michigan and Voyageurs National Park, Minnesota show spatial patterns of depletion of total Hg, organic C, Se, total S, P, and Pb within areas of severe, stand-replacing wildfires that burned in 1936, approximately 65 years prior to our current study. The fires burned during a regional drought, were of high severity, and likely consumed a high percentage of organic forest-floor material (O-horizon). A "fire factor" is defined by positive correlations among Hg, C, Se, S, P, and Pb. A factor score for this six-element grouping derived from factor analysis was assigned to each sample. The scores show a high spatial correlation with the footprint of the 1936 fires in both parks, particularly for A-horizon soils. Because many of these elements are volatile, and are highly correlated with soil organic matter, observed depletions likely represent instantaneous atmospheric release during combustion of O-horizon soils coupled with decades-long reduction of organic matter on the forest floor and near-surface soils. Nearly complete combustion of the modern O-horizon would release roughly 1 mg Hg/m2 from the forest floor. Decades-long disturbance resulting from destruction of mature forests and gradual regrowth following fire also play an important role in Hg cycling. Destruction of a mature forest results in decreased deposition of Hg from litterfall as well as throughfall, which contributes Hg by wash-off of dry deposited Hg from foliar surfaces. Hg in forest soils may follow a fire-dependent cycle in which sudden Hg loss during fire is followed by a period of continued Hg loss as evasion exceeds sequestration in the early stand-replacement stage, finally to resume gradual buildup in later stages of forest regrowth. In the Lake Superior region this cycle exceeds 65 years in duration and is of the same magnitude as the fire return interval for this region. Forests that are controlled by fire-induced cycles of stand replacement may also be in continuous cycles of Hg sequestration and emission. Fire history appears to be a major determinant in the amount of Hg stored in forest soils. Fire almost certainly releases Hg to the atmosphere as forest floor material is burned and thus contributes to atmospheric Hg loads. Fire also appears to cleanse burned areas of Hg both by the atmospheric release during combustion and longer-term release during post-fire forest reorganization. Fire cleansing appears to persist for decades after severe fires and may ameliorate Hg contamination of aquatic food webs by decreasing the soil Hg load of burned watersheds.

Land-Ocean-Atmospheric Coupling Associated with Earthquakes

NASA Astrophysics Data System (ADS)

Prasad, A. K.; Singh, R. P.; Kumar, S.; Cervone, G.; Kafatos, M.; Zlotnicki, J.

2007-12-01

Earthquakes are well known to occur along the plate boundaries and also on the stable shield. The recent studies have shown existence of strong coupling between land-ocean-atmospheric parameters associated with the earthquakes. We have carried out detailed analysis of multi sensor data (optical and microwave remote) to show existence of strong coupling between land-ocean-atmospheric parameters associated with the earthquakes with focal depth up to 30 km and magnitude greater than 5.5. Complimentary nature of various land, ocean and atmospheric parameters will be demonstrated in getting an early warning information about an impending earthquake.

Application of the Approximate Bayesian Computation methods in the stochastic estimation of atmospheric contamination parameters for mobile sources

NASA Astrophysics Data System (ADS)

Kopka, Piotr; Wawrzynczak, Anna; Borysiewicz, Mieczyslaw

2016-11-01

In this paper the Bayesian methodology, known as Approximate Bayesian Computation (ABC), is applied to the problem of the atmospheric contamination source identification. The algorithm input data are on-line arriving concentrations of the released substance registered by the distributed sensors network. This paper presents the Sequential ABC algorithm in detail and tests its efficiency in estimation of probabilistic distributions of atmospheric release parameters of a mobile contamination source. The developed algorithms are tested using the data from Over-Land Atmospheric Diffusion (OLAD) field tracer experiment. The paper demonstrates estimation of seven parameters characterizing the contamination source, i.e.: contamination source starting position (x,y), the direction of the motion of the source (d), its velocity (v), release rate (q), start time of release (ts) and its duration (td). The online-arriving new concentrations dynamically update the probability distributions of search parameters. The atmospheric dispersion Second-order Closure Integrated PUFF (SCIPUFF) Model is used as the forward model to predict the concentrations at the sensors locations.

Investigation of the daytime lunar atmosphere for lunar synthesis program

NASA Technical Reports Server (NTRS)

Hodges, R. R., Jr.

1976-01-01

Synthesis studies of the daytime lunar atmoshere were directed toward improved understanding of fundamental lunar atmospheric dynamics and the relationship of the detectable atmosphere to physical processes of the lunar surface and interior. The primary source of data is the Apollo 17 lunar surface mass spectrometer. The Ar40 is radiogenic and its escape rate from the lunar atmosphere requires release of a significant fraction (about 8%) of the argon produced from the decay of K40 within the moon. Furthermore the process of argon release from the solid moon is time varying and related to seismic activity. Most of the helium on the moon is due to release of implanted solar wind alpha particles from the regolith.

The Influence of Midlatitude Ocean-Atmosphere Coupling on the Low-Frequency Variability of a GCM. Part I: No Tropical SST Forcing*.

NASA Astrophysics Data System (ADS)

Bladé, Ileana

1997-08-01

This study examines the extent to which the thermodynamic interactions between the midlatitude atmosphere and the underlying oceanic mixed layer contribute to the low-frequency atmospheric variability. A general circulation model, run under perpetual northern winter conditions, is coupled to a motionless constant-depth mixed layer in midlatitudes, while elsewhere the sea surface temperature (SST) is kept fixed; interannual tropical SST forcing is not included. It is found that coupling does not modify the spatial organization of the variability. The influence of coupling is manifested as a slight reddening of the spectrum of 500-mb geopotential height and a significant enhancement of the lower-tropospheric thermal variance over the oceans at very low frequencies by virtue of the mixed-layer adjustment to surface air temperature variations that occurs on those timescales. This adjustment effectively reduces the thermal damping of the atmosphere associated with surface heat fluxes (or negative oceanic feedback), thus increasing the thermal variance and the persistence of circulation anomalies.In studying the covariability between ocean and atmosphere it is found that the dominant mode of natural atmospheric variability is coupled to the leading mode of SST in each ocean, with the atmosphere leading the ocean by about one month. The cross-correlation function between oceanic and atmospheric anomalies is strongly asymmetric about zero lag. The SST structures are consistent with direct forcing by the anomalous heat fluxes implied by the concurrent surface air temperature and wind fluctuations. Additionally, composites based on large amplitude SST anomaly events contain no evidence of direct driving of atmospheric perturbations by these SST anomalies. Thus, in terms of the spatial organization of the covariability and the evolution of the coupled system from one regime to another, large-scale air-sea interaction in the model is characterized by one-way atmospheric forcing of the mixed layer.These results are qualitatively consistent with those from an earlier idealized study. They imply a subtle but fundamental role for the midlatitude oceans as stabilizing rather than directly generating atmospheric anomalies. It is argued that this scenario is relevant to the dynamics of extratropical atmosphere-ocean coupling on intraseasonal timescales at least: the model is able to qualitatively reproduce the temporal and spatial characteristics of the observed dominant patterns of interaction on these timescales, particularly over the Atlantic.

Reconstruction of 137Cs activity in the ocean following the Fukushima Daiichi Nuclear Power Plant Accident

NASA Astrophysics Data System (ADS)

Tsumune, Daisuke; Aoyama, Michio; Tsubono, Takaki; Tateda, Yutaka; Misumi, Kazuhiro; Hayami, Hiroshi; Toyoda, Yasuhiro; Maeda, Yoshiaki; Yoshida, Yoshikatsu; Uematsu, Mitsuo

2014-05-01

A series of accidents at the Fukushima Dai-ichi Nuclear Power Plant following the earthquake and tsunami of 11 March 2011 resulted in the release of radioactive materials to the ocean by two major pathways, direct release from the accident site and atmospheric deposition. We reconstructed spatiotemporal variability of 137Cs activity in the ocean by the comparison model simulations and observed data. We employed a regional scale and the North Pacific scale oceanic dispersion models, an atmospheric transport model, a sediment transport model, a dynamic biological compartment model for marine biota and river runoff model to investigate the oceanic contamination. Direct releases of 137Cs were estimated for more than 2 years after the accident by comparing simulated results and observed activities very close to the site. The estimated total amounts of directly released 137Cs was 3.6±0.7 PBq. Directly release rate of 137Cs decreased exponentially with time by the end of December 2012 and then, was almost constant. The daily release rate of 137Cs was estimated to be 3.0 x 1010 Bq day-1 by the end of September 2013. The activity of directly released 137Cs was detectable only in the coastal zone after December 2012. Simulated 137Cs activities attributable to direct release were in good agreement with observed activities, a result that implies the estimated direct release rate was reasonable, while simulated 137Cs activities attributable to atmospheric deposition were low compared to measured activities. The rate of atmospheric deposition onto the ocean was underestimated because of a lack of measurements of dose rate and air activity of 137Cs over the ocean when atmospheric deposition rates were being estimated. Observed 137Cs activities attributable to atmospheric deposition in the ocean helped to improve the accuracy of simulated atmospheric deposition rates. Although there is no observed data of 137Cs activity in the ocean from 11 to 21 March 2011, observed data of marine biota should reflect the history of 137Cs activity in this early period. The comparisons between simulated 137Cs activity of marine biota by a dynamic biological compartment and observed data also suggest that simulated 137Cs activity attributable to atmospheric deposition was underestimated in this early period. In addition, river runoff model simulations suggest that the river flux of 137Cs to the ocean was effective to the 137Cs activity in the ocean in this early period. The sediment transport model simulations suggests that the inventory of 137Cs in sediment was less than 10

Mars Global Reference Atmospheric Model (Mars-GRAM): Release No. 2 - Overview and applications

NASA Technical Reports Server (NTRS)

James, B.; Johnson, D.; Tyree, L.

1993-01-01

The Mars Global Reference Atmospheric Model (Mars-GRAM), a science and engineering model for empirically parameterizing the temperature, pressure, density, and wind structure of the Martian atmosphere, is described with particular attention to the model's newest version, Mars-GRAM, Release No. 2 and to the improvements incorporated into the Release No. 2 model as compared with the Release No. 1 version. These improvements include (1) an addition of a new capability to simulate local-scale Martian dust storms and the growth and decay of these storms; (2) an addition of the Zurek and Haberle (1988) wave perturbation model, for simulating tidal perturbation effects; and (3) a new modular version of Mars-GRAM, for incorporation as a subroutine into other codes.

What the diurnal cycle of precipitation tells us about land-atmosphere coupling strength

NASA Astrophysics Data System (ADS)

Ferguson, Craig; Song, Hyojong; Roundy, Joshua

2015-04-01

The key attributes of a coupled forecast model are the coupling strengths between the land-atmosphere and ocean-atmosphere schemes. If a model cannot skillfully capture the diurnal cycle of clouds and precipitation, then it likely cannot be expected to yield accurate long-term climate projections. The seasonal drought forecast skill shortfalls of the U.S. NCEP Coupled Forecast System Version 2 (CFSv2) have been directly linked to its unrealistically strong land-atmosphere coupling strength. Most models can be similarly categorized, which is to say, sensitivity to the land physics (i.e., soil moisture constraints on evapotranspiration) is too strong. In nature, the land signal: noise ratio appears to be at a much lower value. Diagnosing land-atmosphere coupling strength requires at a minimum: surface soil moisture state, surface turbulent heat fluxes, and atmospheric moisture and instability. Full-on diagnosis would entail hacking into the code and inserting a number of tracers. This study addresses the question: What if, given the soil wetness anomaly, model biases in coupling sign and/or strength could be diagnosed from phase shifts in the diurnal precipitation frequency cycle? We use 34-years of output from the North American Regional Reanalysis (NARR) and North American Land Data Assimilation System Phase 2 (NLDAS-2) to investigate the variation in diurnal precipitation frequency cycle between so-called "wet-advantage" and "dry-advantage" coupling regimes over the U.S. southern Great Plains. Wet-advantage occurs when the atmospheric state is closer to the wet adiabatic rate and convection is triggered by a strong increase in the moist static energy from the surface. In contrast, dry-advantage occurs when the atmosphere is drier and the temperature profile is close to the dry adiabatic lapse rate, which favors convection over areas of large boundary layer growth due to high sensible heat fluxes at the surface. We find that there is a significant difference in the phase of the diurnal precipitation frequency between coupling regimes. Specifically, maximum frequency occurs at 1600 LT and 0500 LT for wet- and dry-advantage samples, respectively. For each of these contrasting regimes, we investigate the relative extent to which diurnal phasing may be attributed to local land -- PBL processes versus influences of the Great Plains low-level jet and large-scale atmospheric circulation.

Session on coupled atmospheric/chemistry coupled models

NASA Technical Reports Server (NTRS)

Thompson, Anne

1993-01-01

The session on coupled atmospheric/chemistry coupled models is reviewed. Current model limitations, current issues and critical unknowns, and modeling activity are addressed. Specific recommendations and experimental strategies on the following are given: multiscale surface layer - planetary boundary layer - chemical flux measurements; Eulerian budget study; and Langrangian experiment. Nonprecipitating cloud studies, organized convective systems, and aerosols - heterogenous chemistry are also discussed.

ESTIMATING GASEOUS EXCHANGES BETWEEN THE ATMOSPHERE AND PLANTS USING A COUPLED BIOCHEMICAL DRY DEPOSITION MODEL

EPA Science Inventory

To study gaseous exchanges between the soil, biosphere and atmosphere, a biochemical model was coupled with the latest version of Meyers Multi-Layer Deposition Model. The biochemical model describes photosynthesis and respiration and their coupling with stomatal resistance for...

Modeling of the dispersion of depleted uranium aerosol.

PubMed

Mitsakou, C; Eleftheriadis, K; Housiadas, C; Lazaridis, M

2003-04-01

Depleted uranium is a low-cost radioactive material that, in addition to other applications, is used by the military in kinetic energy weapons against armored vehicles. During the Gulf and Balkan conflicts concern has been raised about the potential health hazards arising from the toxic and radioactive material released. The aerosol produced during impact and combustion of depleted uranium munitions can potentially contaminate wide areas around the impact sites or can be inhaled by civilians and military personnel. Attempts to estimate the extent and magnitude of the dispersion were until now performed by complex modeling tools employing unclear assumptions and input parameters of high uncertainty. An analytical puff model accommodating diffusion with simultaneous deposition is developed, which can provide a reasonable estimation of the dispersion of the released depleted uranium aerosol. Furthermore, the period of the exposure for a given point downwind from the release can be estimated (as opposed to when using a plume model). The main result is that the depleted uranium mass is deposited very close to the release point. The deposition flux at a couple of kilometers from the release point is more than one order of magnitude lower than the one a few meters near the release point. The effects due to uncertainties in the key input variables are addressed. The most influential parameters are found to be atmospheric stability, height of release, and wind speed, whereas aerosol size distribution is less significant. The output from the analytical model developed was tested against the numerical model RPM-AERO. Results display satisfactory agreement between the two models.

On inter-hemispheric coupling in the middle atmosphere

NASA Astrophysics Data System (ADS)

Karlsson, Bodil; Bailey, S.; Benze, S.; Gumbel, J.; Harvey, V. L.; Kürnich, H.; Lossow, S.; McLandress, D. Marsh, C.; Merkel, A. W.; Mills, M.; Randall, C. E.; Russell, J.; Shepherd, T. G.

On inter-hemispheric coupling in the middle atmosphere From recent studies it is evident that planetary wave activity in the winter hemisphere influences the high-latitude summer mesosphere on the opposite side of the globe. This is an extraordinary example of multi-scale wave-mean flow interaction. The first indication of this inter-hemispheric coupling came from a model study by Becker and Schmitz (2003). Since then, the results have been reproduced in several models, and observations have confirmed the existence of this link. We present current understanding of inter-hemispheric coupling and its consequences for the middle atmosphere, focusing on the summer mesosphere where polar mesospheric clouds (PMCs) form. The results shown are based on year-to-year and intra-seasonal variability in PMCs ob-served by the Odin satellite and the Aeronomy of Ice in the Mesosphere (AIM) satellite, as well as on model results from the extended Canadian Middle Atmosphere Model (CMAM), the Whole Atmosphere Community Climate Model (WACCM) and the Kühlungsborn Mechanis-u tic general Circulation Model (KMCM). The latter has been used to pinpoint the proposed mechanism behind the inter-hemispheric coupling.

Sugarcane vinasse CO2 gasification and release of ash-forming matters in CO2 and N2 atmospheres.

PubMed

Dirbeba, Meheretu Jaleta; Brink, Anders; DeMartini, Nikolai; Lindberg, Daniel; Hupa, Mikko

2016-10-01

Gasification of sugarcane vinasse in CO2 and the release of ash-forming matters in CO2 and N2 atmospheres were investigated using a differential scanning calorimetry and thermogravimetric analyzer (DSC-TGA) at temperatures between 600 and 800°C. The results showed that pyrolysis is the main mechanism for the release of the organics from vinasse. Release of ash-forming matters in the vinasse is the main cause for vinasse char weight losses in the TGA above 700°C. The losses are higher in N2 than in CO2, and increase considerably with temperature. CO2 gasification also consumes the carbon in the vinasse chars while suppressing alkali release. Alkali release was also significant due to volatilization of KCl and reduction of alkali sulfate and carbonate by carbon. The DSC measured thermal events during heating up in N2 atmosphere that correspond to predicted melting temperatures of alkali salts in the char. Copyright © 2016 Elsevier Ltd. All rights reserved.

Modeling and Visualizing Flow of Chemical Agents Across Complex Terrain

NASA Technical Reports Server (NTRS)

Kao, David; Kramer, Marc; Chaderjian, Neal

2005-01-01

Release of chemical agents across complex terrain presents a real threat to homeland security. Modeling and visualization tools are being developed that capture flow fluid terrain interaction as well as point dispersal downstream flow paths. These analytic tools when coupled with UAV atmospheric observations provide predictive capabilities to allow for rapid emergency response as well as developing a comprehensive preemptive counter-threat evacuation plan. The visualization tools involve high-end computing and massive parallel processing combined with texture mapping. We demonstrate our approach across a mountainous portion of North California under two contrasting meteorological conditions. Animations depicting flow over this geographical location provide immediate assistance in decision support and crisis management.

Strong atmospheric chemistry feedback to climate warming from Arctic methane emissions

USGS Publications Warehouse

Isaksen, Ivar S.A.; Gauss, Michael; Myhre, Gunnar; Walter Anthony, Katey M.; Ruppel, Carolyn

2011-01-01

The magnitude and feedbacks of future methane release from the Arctic region are unknown. Despite limited documentation of potential future releases associated with thawing permafrost and degassing methane hydrates, the large potential for future methane releases calls for improved understanding of the interaction of a changing climate with processes in the Arctic and chemical feedbacks in the atmosphere. Here we apply a “state of the art” atmospheric chemistry transport model to show that large emissions of CH4 would likely have an unexpectedly large impact on the chemical composition of the atmosphere and on radiative forcing (RF). The indirect contribution to RF of additional methane emission is particularly important. It is shown that if global methane emissions were to increase by factors of 2.5 and 5.2 above current emissions, the indirect contributions to RF would be about 250% and 400%, respectively, of the RF that can be attributed to directly emitted methane alone. Assuming several hypothetical scenarios of CH4 release associated with permafrost thaw, shallow marine hydrate degassing, and submarine landslides, we find a strong positive feedback on RF through atmospheric chemistry. In particular, the impact of CH4 is enhanced through increase of its lifetime, and of atmospheric abundances of ozone, stratospheric water vapor, and CO2 as a result of atmospheric chemical processes. Despite uncertainties in emission scenarios, our results provide a better understanding of the feedbacks in the atmospheric chemistry that would amplify climate warming.

Antarctic warming driven by internal Southern Ocean deep convection oscillations

NASA Astrophysics Data System (ADS)

Martin, Torge; Pedro, Joel B.; Steig, Eric J.; Jochum, Markus; Park, Wonsun; Rasmussen, Sune O.

2016-04-01

Simulations with the free-running, complex coupled Kiel Climate Model (KCM) show that heat release associated with recurring Southern Ocean deep convection can drive centennial-scale Antarctic temperature variations of 0.5-2.0 °C. We propose a mechanism connecting the intrinsic ocean variability with Antarctic warming that involves the following three steps: Preconditioning: heat supplied by the lower branch of the Atlantic Meridional Overturning Circulation (AMOC) accumulates at depth in the Southern Ocean, trapped by the Weddell Gyre circulation; Convection onset: wind and/or sea-ice changes tip the preconditioned, thermally unstable system into the convective state; Antarctic warming: fast sea-ice-albedo feedbacks (on annual to decadal timescales) and slower Southern Ocean frontal and sea-surface temperature adjustments to the convective heat release (on multi-decadal to centennial timescales), drive an increase in atmospheric heat and moisture transport towards Antarctica resulting in warming over the continent. Further, we discuss the potential role of this mechanism to explain climate variability observed in Antarctic ice-core records.

Thermal Radiation Anomalies Associated with Major Earthquakes

NASA Technical Reports Server (NTRS)

Ouzounov, Dimitar; Pulinets, Sergey; Kafatos, Menas C.; Taylor, Patrick

2017-01-01

Recent developments of remote sensing methods for Earth satellite data analysis contribute to our understanding of earthquake related thermal anomalies. It was realized that the thermal heat fluxes over areas of earthquake preparation is a result of air ionization by radon (and other gases) and consequent water vapor condensation on newly formed ions. Latent heat (LH) is released as a result of this process and leads to the formation of local thermal radiation anomalies (TRA) known as OLR (outgoing Longwave radiation, Ouzounov et al, 2007). We compare the LH energy, obtained by integrating surface latent heat flux (SLHF) over the area and time with released energies associated with these events. Extended studies of the TRA using the data from the most recent major earthquakes allowed establishing the main morphological features. It was also established that the TRA are the part of more complex chain of the short-term pre-earthquake generation, which is explained within the framework of a lithosphere-atmosphere coupling processes.

Hydrometeorology as an Inversion Problem: Can River Discharge Observations Improve the Atmosphere by Ensemble Data Assimilation?

NASA Astrophysics Data System (ADS)

Sawada, Yohei; Nakaegawa, Tosiyuki; Miyoshi, Takemasa

2018-01-01

We examine the potential of assimilating river discharge observations into the atmosphere by strongly coupled river-atmosphere ensemble data assimilation. The Japan Meteorological Agency's Non-Hydrostatic atmospheric Model (JMA-NHM) is first coupled with a simple rainfall-runoff model. Next, the local ensemble transform Kalman filter is used for this coupled model to assimilate the observations of the rainfall-runoff model variables into the JMA-NHM model variables. This system makes it possible to do hydrometeorology backward, i.e., to inversely estimate atmospheric conditions from the information of river flows or a flood on land surfaces. We perform a proof-of-concept Observing System Simulation Experiment, which reveals that the assimilation of river discharge observations into the atmospheric model variables can improve the skill of the short-term severe rainfall forecast.

Seasonally different carbon flux changes in the Southern Ocean in response to the southern annular mode.

PubMed

Hauck, J; Völker, C; Wang, T; Hoppema, M; Losch, M; Wolf-Gladrow, D A

2013-12-01

Stratospheric ozone depletion and emission of greenhouse gases lead to a trend of the southern annular mode (SAM) toward its high-index polarity. The positive phase of the SAM is characterized by stronger than usual westerly winds that induce changes in the physical carbon transport. Changes in the natural carbon budget of the upper 100 m of the Southern Ocean in response to a positive SAM phase are explored with a coupled ecosystem-general circulation model and regression analysis. Previously overlooked processes that are important for the upper ocean carbon budget during a positive SAM period are identified, namely, export production and downward transport of carbon north of the polar front (PF) as large as the upwelling in the south. The limiting micronutrient iron is brought into the surface layer by upwelling and stimulates phytoplankton growth and export production but only in summer. This leads to a drawdown of carbon and less summertime outgassing (or more uptake) of natural CO 2 . In winter, biological mechanisms are inactive, and the surface ocean equilibrates with the atmosphere by releasing CO 2 . In the annual mean, the upper ocean region south of the PF loses more carbon by additional export production than by the release of CO 2 into the atmosphere, highlighting the role of the biological carbon pump in response to a positive SAM event.

Development and validation of a regional coupled forecasting system for S2S forecasts

NASA Astrophysics Data System (ADS)

Sun, R.; Subramanian, A. C.; Hoteit, I.; Miller, A. J.; Ralph, M.; Cornuelle, B. D.

2017-12-01

Accurate and efficient forecasting of oceanic and atmospheric circulation is essential for a wide variety of high-impact societal needs, including: weather extremes; environmental protection and coastal management; management of fisheries, marine conservation; water resources; and renewable energy. Effective forecasting relies on high model fidelity and accurate initialization of the models with observed state of the ocean-atmosphere-land coupled system. A regional coupled ocean-atmosphere model with the Weather Research and Forecasting (WRF) model and the MITGCM ocean model coupled using the ESMF (Earth System Modeling Framework) coupling framework is developed to resolve mesoscale air-sea feedbacks. The regional coupled model allows oceanic mixed layer heat and momentum to interact with the atmospheric boundary layer dynamics at the mesoscale and submesoscale spatiotemporal regimes, thus leading to feedbacks which are otherwise not resolved in coarse resolution global coupled forecasting systems or regional uncoupled forecasting systems. The model is tested in two scenarios in the mesoscale eddy rich Red Sea and Western Indian Ocean region as well as mesoscale eddies and fronts of the California Current System. Recent studies show evidence for air-sea interactions involving the oceanic mesoscale in these two regions which can enhance predictability on sub seasonal timescale. We will present results from this newly developed regional coupled ocean-atmosphere model for forecasts over the Red Sea region as well as the California Current region. The forecasts will be validated against insitu observations in the region as well as reanalysis fields.

Resolving vorticity-driven lateral fire spread using the WRF-Fire coupled atmosphere-fire numerical model

NASA Astrophysics Data System (ADS)

Simpson, C. C.; Sharples, J. J.; Evans, J. P.

2014-09-01

Vorticity-driven lateral fire spread (VLS) is a form of dynamic fire behaviour, during which a wildland fire spreads rapidly across a steep leeward slope in a direction approximately transverse to the background winds. VLS is often accompanied by a downwind extension of the active flaming region and intense pyro-convection. In this study, the WRF-Fire (WRF stands for Weather Research and Forecasting) coupled atmosphere-fire model is used to examine the sensitivity of resolving VLS to both the horizontal and vertical grid spacing, and the fire-to-atmosphere coupling from within the model framework. The atmospheric horizontal and vertical grid spacing are varied between 25 and 90 m, and the fire-to-atmosphere coupling is either enabled or disabled. At high spatial resolutions, the inclusion of fire-to-atmosphere coupling increases the upslope and lateral rate of spread by factors of up to 2.7 and 9.5, respectively. This increase in the upslope and lateral rate of spread diminishes at coarser spatial resolutions, and VLS is not modelled for a horizontal and vertical grid spacing of 90 m. The lateral fire spread is driven by fire whirls formed due to an interaction between the background winds and the vertical circulation generated at the flank of the fire front as part of the pyro-convective updraft. The laterally advancing fire fronts become the dominant contributors to the extreme pyro-convection. The results presented in this study demonstrate that both high spatial resolution and two-way atmosphere-fire coupling are required to model VLS with WRF-Fire.

Effects of explicit convection on global land-atmosphere coupling in the superparameterized CAM

NASA Astrophysics Data System (ADS)

Sun, Jian; Pritchard, Michael S.

2016-09-01

Conventional global climate models are prone to producing unrealistic land-atmosphere coupling signals. Cumulus and convection parameterizations are natural culprits but the effect of bypassing them with explicitly resolved convection on global land-atmosphere coupling dynamics has not been explored systematically. We apply a suite of modern land-atmosphere coupling diagnostics to isolate the effect of cloud Superparameterization in the Community Atmosphere Model (SPCAM) v3.5, focusing on both the terrestrial segment (i.e., soil moisture and surface turbulent fluxes interaction) and atmospheric segment (i.e., surface turbulent fluxes and precipitation interaction) in the water pathway of the land-atmosphere feedback loop. At daily timescales, SPCAM produces stronger uncoupled terrestrial signals (negative sign) over tropical rainforests in wet seasons, reduces the terrestrial coupling strength in the Central Great Plain in American, and reverses the coupling sign (from negative to positive) over India in the boreal summer season—all favorable improvements relative to reanalysis-forced land modeling. Analysis of the triggering feedback strength (TFS) and amplification feedback strength (AFS) shows that SPCAM favorably reproduces the observed geographic patterns of these indices over North America, with the probability of afternoon precipitation enhanced by high evaporative fraction along the eastern United States and Mexico, while conventional CAM does not capture this signal. We introduce a new diagnostic called the Planetary Boundary Layer (PBL) Feedback Strength (PFS), which reveals that SPCAM exhibits a tight connection between the responses of the lifting condensation level, the PBL height, and the rainfall triggering to surface turbulent fluxes; a triggering disconnect is found in CAM.

Quantifying the Role of Atmospheric Forcing in Ice Edge Retreat and Advance Including Wind-Wave Coupling

DTIC Science & Technology

2015-09-30

Quantifying the Role of Atmospheric Forcing in Ice Edge Retreat and Advance Including Wind- Wave Coupling Peter S. Guest (NPS Technical Contact) Naval...surface fluxes and ocean waves in coupled models in the Beaufort and Chukchi Seas. 2. Understand the physics of heat and mass transfer from the ocean...to the atmosphere. 3. Improve forecasting of waves on the open ocean and in the marginal ice zone. 2 OBJECTIVES 1. Quantifying the open-ocean

Global Effects of Superparameterization on Hydrothermal Land-Atmosphere Coupling on Multiple Timescales

NASA Astrophysics Data System (ADS)

Qin, Hongchen; Pritchard, Michael S.; Kooperman, Gabriel J.; Parishani, Hossein

2018-02-01

Many conventional General Circulation Models (GCMs) in the Global Land-Atmosphere Coupling Experiment (GLACE) tend to produce what is now recognized as overly strong land-atmosphere (L-A) coupling. We investigate the effects of cloud Superparameterization (SP) on L-A coupling on timescales beyond diurnal where it has been recently shown to have a favorable muting effect hydrologically. Using the Community Atmosphere Model v3.5 (CAM3.5) and its Superparameterized counterpart SPCAM3.5, we conducted soil moisture interference experiments following the GLACE and Atmospheric Model Intercomparison Project (AMIP) protocols. The results show that, on weekly-to-subseasonal timescales, SP also mutes hydrologic L-A coupling. This is detectable globally, and happens through the evapotranspiration-precipitation segment. But on seasonal timescales, SP does not exhibit detectable effects on hydrologic L-A coupling. Two robust regional effects of SP on thermal L-A coupling have also been explored. Over the Arabian Peninsula, SP reduces thermal L-A coupling through a straightforward control by mean rainfall reduction. More counterintuitively, over the Southwestern US and Northern Mexico, SP enhances the thermal L-A coupling in a way that is independent of rainfall and soil moisture. This signal is associated with a systematic and previously unrecognized effect of SP that produces an amplified Bowen ratio, and is detectable in multiple SP model versions and experiment designs. In addition to amplifying the present-day Bowen ratio, SP is found to amplify the climate sensitivity of Bowen ratio as well, which likely plays a role in influencing climate change predictions at the L-A interface.

Climate Simulations based on a different-grid nested and coupled model

NASA Astrophysics Data System (ADS)

Li, Dan; Ji, Jinjun; Li, Yinpeng

2002-05-01

An atmosphere-vegetation interaction model (A VIM) has been coupled with a nine-layer General Cir-culation Model (GCM) of Institute of Atmospheic Physics/State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics (IAP/LASG), which is rhomboidally truncated at zonal wave number 15, to simulate global climatic mean states. A VIM is a model having inter-feedback between land surface processes and eco-physiological processes on land. As the first step to couple land with atmosphere completely, the physiological processes are fixed and only the physical part (generally named the SVAT (soil-vegetation-atmosphere-transfer scheme) model) of AVIM is nested into IAP/LASG L9R15 GCM. The ocean part of GCM is prescribed and its monthly sea surface temperature (SST) is the climatic mean value. With respect to the low resolution of GCM, i.e., each grid cell having lon-gitude 7.5° and latitude 4.5°, the vegetation is given a high resolution of 1.5° by 1.5° to nest and couple the fine grid cells of land with the coarse grid cells of atmosphere. The coupling model has been integrated for 15 years and its last ten-year mean of outputs was chosen for analysis. Compared with observed data and NCEP reanalysis, the coupled model simulates the main characteris-tics of global atmospheric circulation and the fields of temperature and moisture. In particular, the simu-lated precipitation and surface air temperature have sound results. The work creates a solid base on coupling climate models with the biosphere.

Representative Atmospheric Plume Development for Elevated Releases

DOE Office of Scientific and Technical Information (OSTI.GOV)

Eslinger, Paul W.; Lowrey, Justin D.; McIntyre, Justin I.

2014-02-01

An atmospheric explosion of a low-yield nuclear device will produce a large number of radioactive isotopes, some of which can be measured with airborne detection systems. However, properly equipped aircraft may not arrive in the region where an explosion occurred for a number of hours after the event. Atmospheric conditions will have caused the radioactive plume to move and diffuse before the aircraft arrives. The science behind predicting atmospheric plume movement has advanced enough that the location of the maximum concentrations in the plume can be determined reasonably accurately in real time, or near real time. Given the assumption thatmore » an aircraft can follow a plume, this study addresses the amount of atmospheric dilution expected to occur in a representative plume as a function of time past the release event. The approach models atmospheric transport of hypothetical releases from a single location for every day in a year using the publically available HYSPLIT code. The effective dilution factors for the point of maximum concentration in an elevated plume based on a release of a non-decaying, non-depositing tracer can vary by orders of magnitude depending on the day of the release, even for the same number of hours after the release event. However, the median of the dilution factors based on releases for 365 consecutive days at one site follows a power law relationship in time, as shown in Figure S-1. The relationship is good enough to provide a general rule of thumb for estimating typical future dilution factors in a plume starting at the same point. However, the coefficients of the power law function may vary for different release point locations. Radioactive decay causes the effective dilution factors to decrease more quickly with the time past the release event than the dilution factors based on a non-decaying tracer. An analytical expression for the dilution factors of isotopes with different half-lives can be developed given the power law expression for the non-decaying tracer. If the power-law equation for the median dilution factor, Df, based on a non-decaying tracer has the general form Df=a(×t)^(-b) for time t after the release event, then the equation has the form Df=e^(-λt)×a×t^(-b) for a radioactive isotope, where λ is the decay constant for the isotope.« less

Release of ethanol to the atmosphere during use of consumer cleaning products

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wooley, J.; Nazaroff, W.W.; Hodgson, A.T.

1990-08-01

Liquid laundry and hand dish washing detergents contain volatile organic compounds, including ethanol, that may be liberated during use and contribute to photochemical air pollution. In this study, the release of ethanol to the atmosphere during simulated household use of liquid detergents was measured. Three replicate experiments, plus a blank, were conducted in a 20-m{sup 3} environmental chamber for each of four conditions: typical dish washing (DT), high-release dish washing (DH), typical laundry (LT), and high-release laundry (LH). Average amounts of ethanol transferred to the atmosphere per use (and the fraction of ethanol used so liberated) were 32 mg (0.038)more » for DT, 100 mg (0.049) for DH, 18 mg (0.002) for LT, and 110 mg (0.011) for LH. Thus, a large fraction of the ethanol added to wash solutions with liquid detergents is discharged to the sewer rather than transferred to the atmosphere during use.« less

A New Approach for Coupled GCM Sensitivity Studies

NASA Astrophysics Data System (ADS)

Kirtman, B. P.; Duane, G. S.

2011-12-01

A new multi-model approach for coupled GCM sensitivity studies is presented. The purpose of the sensitivity experiments is to understand why two different coupled models have such large differences in their respective climate simulations. In the application presented here, the differences between the coupled models using the Center for Ocean-Land-Atmosphere Studies (COLA) and the National Center for Atmospheric Research (NCAR) atmospheric general circulation models (AGCMs) are examined. The intent is to isolate which component of the air-sea fluxes is most responsible for the differences between the coupled models and for the errors in their respective coupled simulations. The procedure is to simultaneously couple the two different atmospheric component models to a single ocean general circulation model (OGCM), in this case the Modular Ocean Model (MOM) developed at the Geophysical Fluid Dynamics Laboratory (GFDL). Each atmospheric component model experiences the same SST produced by the OGCM, but the OGCM is simultaneously coupled to both AGCMs using a cross coupling strategy. In the first experiment, the OGCM is coupled to the heat and fresh water flux from the NCAR AGCM (Community Atmospheric Model; CAM) and the momentum flux from the COLA AGCM. Both AGCMs feel the same SST. In the second experiment, the OGCM is coupled to the heat and fresh water flux from the COLA AGCM and the momentum flux from the CAM AGCM. Again, both atmospheric component models experience the same SST. By comparing these two experimental simulations with control simulations where only one AGCM is used, it is possible to argue which of the flux components are most responsible for the differences in the simulations and their respective errors. Based on these sensitivity experiments we conclude that the tropical ocean warm bias in the COLA coupled model is due to errors in the heat flux, and that the erroneous westward shift in the tropical Pacific cold tongue minimum in the NCAR model is due errors in the momentum flux. All the coupled simulations presented here have warm biases along the eastern boundary of the tropical oceans suggesting that the problem is common to both AGCMs. In terms of interannual variability in the tropical Pacific, the CAM momentum flux is responsible for the erroneous westward extension of the sea surface temperature anomalies (SSTA) and errors in the COLA momentum flux cause the erroneous eastward migration of the El Niño-Southern Oscillation (ENSO) events. These conclusions depend on assuming that the error due to the OGCM can be neglected.

The effect of platform switching on the levels of metal ion release from different implant–abutment couples

PubMed Central

Alrabeah, Ghada O; Knowles, Jonathan C; Petridis, Haralampos

2016-01-01

The improved peri-implant bone response demonstrated by platform switching may be the result of reduced amounts of metal ions released to the surrounding tissues. The aim of this study was to compare the levels of metal ions released from platform-matched and platform-switched implant–abutment couples as a result of accelerated corrosion. Thirty-six titanium alloy (Ti-6Al-4V) and cobalt–chrome alloy abutments were coupled with titanium cylinders forming either platform-switched or platform-matched groups (n=6). In addition, 18 unconnected samples served as controls. The specimens were subjected to accelerated corrosion by static immersion in 1% lactic acid for 1 week. The amount of metal ions ion of each test tube was measured using inductively coupled plasma mass spectrometry. Scanning electron microscope (SEM) images and energy dispersive spectroscopy X-ray analyses were performed pre- and post-immersion to assess corrosion at the interface. The platform-matched groups demonstrated higher ion release for vanadium, aluminium, cobalt, chrome, and molybdenum compared with the platform-switched groups (P<0.05). Titanium was the highest element to be released regardless of abutment size or connection (P<0.05). SEM images showed pitting corrosion prominent on the outer borders of the implant and abutment platform surfaces. In conclusion, implant–abutment couples underwent an active corrosion process resulting in metal ions release into the surrounding environment. The highest amount of metal ions released was recorded for the platform-matched groups, suggesting that platform-switching concept has a positive effect in reducing the levels of metal ion release from the implant–abutment couples. PMID:27357323

ATMOSPHERIC RELEASES FROM STANDARDIZED NUCLEAR POWER PLANTS: A WIND TUNNEL STUDY

EPA Science Inventory

Laboratory experiments were conducted to simulate radiopollutant effluents released to the atmosphere from two standard design nuclear power plants. The main objective of the study was to compare the dispersion in the wake of the standardized nuclear power plants with that in a s...

Impacts of Irrigation on Land-Atmosphere Coupling Strength Under Different Evapotranspiration Characteristics

NASA Astrophysics Data System (ADS)

Liao, C. Y.; Lo, M. H.

2017-12-01

The Budyko curve displays that the magnitude of evapotranspiration (ET) is limited mainly by the availabilities of energy and water, i.e., under wet conditions, ET is primarily controlled by the available energy, while under dry conditions, ET is primarily controlled by the available water. Land-atmosphere coupling (LAC) strength, which relates to the Budyko curve, is widely discussed because of its contribution towards the improvement in seasonal climate forecasts. For example, the "hot spots" of LAC, where the soil moisture anomalies strongly affect the local precipitation, are found in the transition zones between wet and dry climates. ET of these transition zones is limited by the available water, but at the same time, the surface latent heat flux is large enough to trigger moist convection. Recently, the impacts of irrigation have gained lots of attention, including the change in LAC. Badger and Dirmeyer (2015) analyzed the climate response of Amazon forest replacement by crop with consideration of irrigation in model simulations, discovering negative relationship between added irrigation water and coupling between the soil moisture and the latent heat flux. In addition, Lu et al. (2017) found remarkable decreases of LAC strength with the increase of irrigated cropland percentage in the Great Plains of America. The two studies show that irrigation is possible to affect land-atmosphere coupling strength. However, whether the irrigation process leads to the reduction of coupling strength in other regions of the world remains unclear. This study aims to compare the differences of irrigation impact on land-atmosphere coupling strength between five selected locations undergoing intense irrigation: India, North China Plain, Southwest Europe, Great Plains and Middle East. The spatial divergence of the factor that limits the ET (e.g., either by the available energy or water) will be the focus in this study. Both offline simulation (Community Land Model) and couple simulation (coupled with Community Atmosphere Model) are used to explore the direct change and the subsequent shifts in land-atmosphere interactions. Also, three LAC indices are adopted to quantify the coupling strength between land and atmosphere.

Predicting Atmospheric Releases from the September 3, 2017 North Korean Event

NASA Astrophysics Data System (ADS)

Lucas, D. D.; Simpson, M. D.; Glascoe, L. G.

2017-12-01

Underground nuclear explosions produce radionuclides that can be vented to the atmosphere and transported to International Monitoring System (IMS) measurement stations. Although a positive atmospheric detection from North Korea's declared test on September 3, 2017 has not been reported at any IMS station through early October, atmospheric transport models can predict when and where detections may arise and provide valuable information to optimize air collection strategies. We present predictive atmospheric transport simulations initiated in the early days after the event. Wind fields were simulated with the Weather Research and Forecast model and used to transport air tracers from an ensemble of releases in the FLEXPART dispersion model. If early venting had occurred, the simulations suggested that detections were possible at the IMS station in Takasaki, Japan. On-going and future research efforts associated with nuclear testing are focused on quantifying meteorological uncertainty, simulating releases in complex terrain, and developing new statistical methods for source attribution. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and is released as LLNL-ABS-740341.

3rd IAGA/ICMA Workshop on Vertical Coupling in the Atmosphere/Ionosphere System/ Abstract

DTIC Science & Technology

2007-01-10

energy and momentum from the lower atmosphere to the upper atmosphere and ionosphere and vice versa. The programme focussed on various aspects and...ICMA Workshop Vertical Coupling in the Atmosphere/Ionosphere System - 6 - The influence of global dependence of gravity wave energy in the troposphere...transport during the polar night of thermospheric odd nitrogen produced by lower- energy electron precipitation and solar extreme UV fluxes. However, at low

Estimations of Atmospheric Conditions for Input to the Radar Performance Surface

DTIC Science & Technology

2007-12-01

timely atmospheric and ocean surface descriptions on features that impact radar and electro-optical sensor systems . The first part of this study is an...Navy’s Coupled Ocean Atmosphere Mesoscale Prediction System (COAMPS®) are compared to in-situ data to assess the sensitivities of air-sea...temperature measurements to make direct comparisons to the Coupled Ocean Atmosphere Mesoscale Prediction System (COAMPS®) as a prime source of input to the

Middle atmospheric electrodynamics

NASA Technical Reports Server (NTRS)

Kelley, M. C.

1983-01-01

A review is presented of the advances made during the last few years with respect to the study of the electrodynamics in the earth's middle atmosphere. In a report of the experimental work conducted, attention is given to large middle atmospheric electric fields, the downward coupling of high altitude processes into the middle atmosphere, and upward coupling of tropospheric processes into the middle atmosphere. It is pointed out that new developments in tethered balloons and superpressure balloons should greatly increase the measurement duration of earth-ionospheric potential measurements and of stratospheric electric field measurements in the next few years. Theoretical work considered provides an excellent starting point for study of upward coupling of transient and dc electric fields. Hays and Roble (1979) were the first to construct a model which included orographic features as well as the classical thunderstorm generator.

Maxine: A spreadsheet for estimating dose from chronic atmospheric radioactive releases

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jannik, Tim; Bell, Evaleigh; Dixon, Kenneth

MAXINE is an EXCEL© spreadsheet, which is used to estimate dose to individuals for routine and accidental atmospheric releases of radioactive materials. MAXINE does not contain an atmospheric dispersion model, but rather doses are estimated using air and ground concentrations as input. Minimal input is required to run the program and site specific parameters are used when possible. Complete code description, verification of models, and user’s manual have been included.

GLACE: The Global Land-Atmosphere Coupling Experiment. Part 1; Overview

NASA Technical Reports Server (NTRS)

Koster, Randal D.; Guo, Zhi-Chang; Dirmeyer, Paul A.; Bonan, Gordon; Chan, Edmond; Cox, Peter; Davies, Harvey; Gordon, C. T.; Kanae, Shinjiro; Kowalczyk, Eva

2005-01-01

GLACE is a model intercomparison study focusing on a typically neglected yet critical element of numerical weather and climate modeling: land-atmosphere coupling strength, or the degree to which anomalies in land surface state (e.g., soil moisture) can affect rainfall generation and other atmospheric processes. The twelve AGCM groups participating in GLACE performed a series of simple numerical experiments that allow the objective quantification of this element. The derived coupling strengths vary widely. Some similarity, however, is found in the spatial patterns generated by the models, enough similarity to pinpoint multi-model "hot spots" of land-atmosphere coupling. For boreal summer, such hot spots for precipitation and temperature are found over large regions of Africa, central North America and India; a hot spot for temperature is also found over eastern China. The design of the GLACE simulations are described in full detail so that any interested modeling group can repeat them easily and thereby place their model s coupling strength within the broad range of those documented here.

Atmosphere, ocean, and land: Critical gaps in Earth system models

NASA Technical Reports Server (NTRS)

Prinn, Ronald G.; Hartley, Dana

1992-01-01

We briefly review current knowledge and pinpoint some of the major areas of uncertainty for the following fundamental processes: (1) convection, condensation nuclei, and cloud formation; (2) oceanic circulation and its coupling to the atmosphere and cryosphere; (3) land surface hydrology and hydrology-vegetation coupling; (4) biogeochemistry of greenhouse gases; and (5) upper atmospheric chemistry and circulation.

Modelling the effect of soil moisture and organic matter degradation on biogenic NO emissions from soils in Sahel rangeland (Mali)

NASA Astrophysics Data System (ADS)

Delon, C.; Mougin, E.; Serça, D.; Grippa, M.; Hiernaux, P.; Diawara, M.; Galy-Lacaux, C.; Kergoat, L.

2015-01-01

This work is an attempt to provide seasonal variation of biogenic NO emission fluxes in a sahelian rangeland in Mali (Agoufou, 15.34° N, 1.48° W) for years 2004-2008. Indeed, NO is one of the most important precursor for tropospheric ozone, and the contribution of the Sahel region in emitting NO is no more considered as negligible. The link between NO production in the soil and NO release to the atmosphere is investigated in this study, by taking into account vegetation litter production and degradation, microbial processes in the soil, emission fluxes, and environmental variables influencing these processes, using a coupled vegetation-litter decomposition-emission model. This model includes the Sahelian-Transpiration-Evaporation-Productivity (STEP) model for the simulation of herbaceous, tree leaf and fecal masses, the GENDEC model (GENeral DEComposition) for the simulation of the buried litter decomposition and microbial dynamics, and the NO emission model (NOFlux) for the simulation of the NO release to the atmosphere. Physical parameters (soil moisture and temperature, wind speed, sand percentage) which affect substrate diffusion and oxygen supply in the soil and influence the microbial activity, and biogeochemical parameters (pH and fertilization rate related to N content) are necessary to simulate the NO flux. The reliability of the simulated parameters is checked, in order to assess the robustness of the simulated NO flux. Simulated yearly average of NO flux ranges from 0.66 to 0.96 kg(N) ha-1 yr-1, and wet season average ranges from 1.06 to 1.73 kg(N) ha-1 yr-1. These results are in the same order as previous measurements made in several sites where the vegetation and the soil are comparable to the ones in Agoufou. This coupled vegetation-litter decomposition-emission model could be generalized at the scale of the Sahel region, and provide information where little data is available.

Storage and on-demand release of microwaves using superconducting resonators with tunable coupling

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pierre, Mathieu, E-mail: mathieu.pierre@lncmi.cnrs.fr; Svensson, Ida-Maria; Raman Sathyamoorthy, Sankar

2014-06-09

We present a system which allows to tune the coupling between a superconducting resonator and a transmission line. This storage resonator is addressed through a second, coupling resonator, which is frequency-tunable and controlled by a magnetic flux applied to a superconducting quantum interference device. We experimentally demonstrate that the lifetime of the storage resonator can be tuned by more than three orders of magnitude. A field can be stored for 18 μs when the coupling resonator is tuned off resonance and it can be released in 14 ns when the coupling resonator is tuned on resonance. The device allows capture, storage, andmore » on-demand release of microwaves at a tunable rate.« less

Atmospheric plume progression as a function of time and distance from the release point for radioactive isotopes.

PubMed

Eslinger, Paul W; Bowyer, Ted W; Cameron, Ian M; Hayes, James C; Miley, Harry S

2015-10-01

The radionuclide network of the International Monitoring System comprises up to 80 stations around the world that have aerosol and xenon monitoring systems designed to detect releases of radioactive materials to the atmosphere from nuclear explosions. A rule of thumb description of plume concentration and duration versus time and distance from the release point is useful when designing and deploying new sample collection systems. This paper uses plume development from atmospheric transport modeling to provide a power-law rule describing atmospheric dilution factors as a function of distance from the release point. Consider the plume center-line concentration seen by a ground-level sampler as a function of time based on a short-duration ground-level release of a nondepositing radioactive tracer. The concentration C (Bq m(-3)) near the ground varies with distance from the source with the relationship C=R×A(D,C) ×e (-λ(-1.552+0.0405×D)) × 5.37×10(-8) × D(-2.35) where R is the release magnitude (Bq), D is the separation distance (km) from the ground level release to the measurement location, λ is the decay constant (h(-1)) for the radionuclide of interest and AD,C is an attenuation factor that depends on the length of the sample collection period. This relationship is based on the median concentration for 10 release locations with different geographic characteristics and 365 days of releases at each location, and it has an R(2) of 0.99 for 32 distances from 100 to 3000 km. In addition, 90 percent of the modeled plumes fall within approximately one order of magnitude of this curve for all distances. Copyright © 2015 Elsevier Ltd. All rights reserved.

How trees uptake carbon, release water and cool themselves in air: a marriage between biophysics and turbulent fluid dynamics

NASA Astrophysics Data System (ADS)

Banerjee, Tirtha; Linn, Rodman

2017-11-01

Resolving the role of the biosphere as a terrestrial carbon sink and the nature of nonlinear couplings between carbon and water cycles across a very wide range of spatiotemporal scales constitute the scope of this work. To achieve this goal, plant physiology models are coupled with atmospheric turbulence simulations. The plant biophysics code is based on the following principles: (1) a model for photosynthesis; (2) a mass transfer model through the laminar boundary layer on leaves; (3) an optimal leaf water use strategy regulated by stomatal aperture variation; (4) a leaf-level energy balance to accommodate evaporative cooling. Leaf-level outputs are upscaled to plant, canopy and landscape scales using HIGRAD/FIRETEC, a high fidelity large eddy simulation (LES) framework developed at LANL. The coupled biophysics-CFD code can take inputs such as wind speed, light availability, ambient CO2 concentration, air temperature, site characteristics etc. and can deliver predictions for leaf temperature, transpiration, carbon assimilation, sensible and latent heat flux, which is used to illustrate the complex the complex interaction between trees and their surrounding environments. These simulation capabilities are being used to study climate feedbacks of forests and agroecosystems.

Air-Sea Momentum and Enthalpy Exchange in Coupled Atmosphere-Wave-Ocean Modeling of Tropical Cyclones

NASA Astrophysics Data System (ADS)

Curcic, M.; Chen, S. S.

2016-02-01

The atmosphere and ocean are coupled through momentum, enthalpy, and mass fluxes. Accurate representation of these fluxes in a wide range of weather and climate conditions is one of major challenges in prediction models. Their current parameterizations are based on sparse observations in low-to-moderate winds and are not suited for high wind conditions such as tropical cyclones (TCs) and winter storms. In this study, we use the Unified Wave INterface - Coupled Model (UWIN-CM), a high resolution, fully-coupled atmosphere-wave-ocean model, to better understand the role of ocean surface waves in mediating air-sea momentum and enthalpy exchange in TCs. In particular, we focus on the explicit treatment of wave growth and dissipation for calculating atmospheric and oceanic stress, and its role in upper ocean mixing and surface cooling in the wake of the storm. Wind-wave misalignment and local wave disequilibrium result in difference between atmospheric and oceanic stress being largest on the left side of the storm. We find that explicit wave calculation in the coupled model reduces momentum transfer into the ocean by more than 10% on average, resulting in reduced cooling in TC's wake and subsequent weakening of the storm. We also investigate the impacts of sea surface temperature and upper ocean parameterization on air-sea enthalpy fluxes in the fully coupled model. High-resolution UWIN-CM simulations of TCs with various intensities and structure are conducted in this study to better understand the complex TC-ocean interaction and improve the representation of air-sea coupling processes in coupled prediction models.

Calculation of temperatures in condensed phase of burning PMMA by equation of Michelson, Mullar and Le Chatelier

NASA Astrophysics Data System (ADS)

Turgumbayeva, R. Kh; Abdikarimov, M. N.; Sagintayeva, S. S.

2018-05-01

Results of studying an aerosol of the dioxide of sulfur and pentoxide of phosphorus released into the atmosphere by the chemical company for processing of phosphorit are presented. Influence of the direction and speed of wind on sulfur dioxide distribution and pentoxide of phosphorus in a ground layer of the atmosphere is studied, and the points of the direction of wind leading to pollution of the atmosphere of the nearby city are allocated. The statistical analysis of environmental pollution is carried out by the method of the correlation and regression analysis. The equations of dependence of the amount of the sulfur dioxide and pentoxide of phosphorus, released into the atmosphere, on the volume, released by the enterprise of production, are defined. The obtained results are recommended for control, regulation and management of the environment.

Middle Atmosphere Electrodynamics During a Thunderstorm

NASA Technical Reports Server (NTRS)

Croskey, Charles L.

1996-01-01

Rocket-based instrumentation investigations of middle atmospheric electrodynamics during thunderstorms were conducted in coordination with balloon-measurements at Wallops Island, Virginia. Middle atmosphere electrodynamics and energy coupling are of particular importance to associated electrical processes at lower and higher altitudes. Objectives of this research effort included: (1) investigation of thunderstorm effects on middle atmosphere electrical structure, including spatial and temporal dependence; (2) characterization of electric field transients and the associated energy deposited at various altitudes; (3) evaluation of the vertical Maxwell current density over a thunderstorm to study the coupling of energy to higher altitudes; and (4) investigation of the coupling of energy to the ionosphere and the current supplied to the 'global circuit.'

Recharge of the early atmosphere of Mars by impact-induced release of CO2

NASA Technical Reports Server (NTRS)

Carr, Michael H.

1989-01-01

The question as to whether high impact rates early in the history of Mars could have aided in maintaining a relatively thick CO2 atmosphere is discussed. Such impacts could have released CO2 into the atmosphere by burial, by shock-induced release during impact events, and by the addition of carbon to Mars from the impacting bolides. On the assumption that cratering rates on Mars were comparable to those of the moon's Nectarial period, burial rates are a result of 'impact gardening' at the end of heavy bombardment are estimated to have ranged from 20 to 45 m/million years; at these rates, 0.1-0.2 bar of CO2 would have been released every 10 million years as a result of burial to depths at which carbonate dissociation temperatures are encountered.

Resolving vorticity-driven lateral fire spread using the WRF-Fire coupled atmosphere-fire numerical model

NASA Astrophysics Data System (ADS)

Simpson, C. C.; Sharples, J. J.; Evans, J. P.

2014-05-01

Fire channelling is a form of dynamic fire behaviour, during which a wildland fire spreads rapidly across a steep lee-facing slope in a direction transverse to the background winds, and is often accompanied by a downwind extension of the active flaming region and extreme pyro-convection. Recent work using the WRF-Fire coupled atmosphere-fire model has demonstrated that fire channelling can be characterised as vorticity-driven lateral fire spread (VDLS). In this study, 16 simulations are conducted using WRF-Fire to examine the sensitivity of resolving VDLS to spatial resolution and atmosphere-fire coupling within the WRF-Fire model framework. The horizontal grid spacing is varied between 25 and 90 m, and the two-way atmosphere-fire coupling is either enabled or disabled. At high spatial resolution, the atmosphere-fire coupling increases the peak uphill and lateral spread rate by a factor of up to 2.7 and 9.5. The enhancement of the uphill and lateral spread rate diminishes at coarser spatial resolution, and VDLS is not modelled for a horizontal grid spacing of 90 m. The laterally spreading fire fronts become the dominant contributors of the extreme pyro-convection. The resolved fire-induced vortices responsible for driving the lateral spread in the coupled simulations have non-zero vorticity along each unit vector direction, and develop due to an interaction between the background winds and vertical return circulations generated at the flank of the fire front as part of the pyro-convective updraft. The results presented in this study demonstrate that both high spatial resolution and two-way atmosphere-fire coupling are required to reproduce VDLS within the current WRF-Fire model framework.

GEWEX SRB Shortwave Release 4

NASA Astrophysics Data System (ADS)

Cox, S. J.; Stackhouse, P. W., Jr.; Mikovitz, J. C.; Zhang, T.

2017-12-01

The NASA/GEWEX Surface Radiation Budget (SRB) project produces shortwave and longwave surface and top of atmosphere radiative fluxes for the 1983-near present time period. Spatial resolution is 1 degree. The new Release 4 uses the newly processed ISCCP HXS product as its primary input for cloud and radiance data. The ninefold increase in pixel number compared to the previous ISCCP DX allows finer gradations in cloud fraction in each grid box. It will also allow higher spatial resolutions (0.5 degree) in future releases. In addition to the input data improvements, several important algorithm improvements have been made since Release 3. These include recalculated atmospheric transmissivities and reflectivities yielding a less transmissive atmosphere. The calculations also include variable aerosol composition, allowing for the use of a detailed aerosol history from the Max Planck Institut Aerosol Climatology (MAC). Ocean albedo and snow/ice albedo are also improved from Release 3. Total solar irradiance is now variable, averaging 1361 Wm-2. Water vapor is taken from ISCCP's nnHIRS product. Results from GSW Release 4 are presented and analyzed. Early comparison to surface measurements show improved agreement.

Safe atmosphere entry of an isotope heat source with a single stable trim attitude at hypersonic speeds

NASA Technical Reports Server (NTRS)

Levy, L. L., Jr.; Burns, R. K.

1972-01-01

A theoretical investigation has been made to design an isotope heat source capable of satisfying the conflicting thermal requirements of steady-state operation and atmosphere entry. The isotope heat source must transfer heat efficiently to a heat exchange during normal operation with a power system in space, and in the event of a mission abort, it must survive the thermal environment of atmosphere entry and ground impact without releasing radioactive material. A successful design requires a compatible integration of the internal components of the heat source with the external aerodynamic shape. To this end, configurational, aerodynamic, motion, and thermal analyses were coupled and iterated during atmosphere entries at suborbital through superorbital velocities at very shallow and very steep entry angles. Results indicate that both thermal requirements can be satisfied by a heat source which has a single stable aerodynamic orientation at hypersonic speeds. For such a design, the insulation material required to adequately protect the isotope fuel from entry heating need extend only half way around the fuel capsule on the aerodynamically stable (wind-ward) side of the heat source. Thus, a low-thermal-resistance, conducting heat path is provided on the opposite side of the heat source through which heat can be transferred to an adjacent heat exchanger during normal operation without exceeding specified temperature limits.

An ensemble Kalman filter with a high-resolution atmosphere-ocean coupled model for tropical cyclone forecasts

NASA Astrophysics Data System (ADS)

Kunii, M.; Ito, K.; Wada, A.

2015-12-01

An ensemble Kalman filter (EnKF) using a regional mesoscale atmosphere-ocean coupled model was developed to represent the uncertainties of sea surface temperature (SST) in ensemble data assimilation strategies. The system was evaluated through data assimilation cycle experiments over a one-month period from July to August 2014, during which a tropical cyclone as well as severe rainfall events occurred. The results showed that the data assimilation cycle with the coupled model could reproduce SST distributions realistically even without updating SST and salinity during the data assimilation cycle. Therefore, atmospheric variables and radiation applied as a forcing to ocean models can control oceanic variables to some extent in the current data assimilation configuration. However, investigations of the forecast error covariance estimated in EnKF revealed that the correlation between atmospheric and oceanic variables could possibly lead to less flow-dependent error covariance for atmospheric variables owing to the difference in the time scales between atmospheric and oceanic variables. A verification of the analyses showed positive impacts of applying the ocean model to EnKF on precipitation forecasts. The use of EnKF with the coupled model system captured intensity changes of a tropical cyclone better than it did with an uncoupled atmosphere model, even though the impact on the track forecast was negligibly small.

Orbit-spin coupling and the circulation of the Martian atmosphere

NASA Astrophysics Data System (ADS)

Shirley, James H.

2017-07-01

The physical origins of the observed interannual variability of weather and climate on Mars are poorly understood. In this paper we introduce a deterministic physical mechanism that may account for much of the variability of the circulation of the Mars atmosphere on seasonal and longer timescales. We focus on a possible coupling between the planetary orbital angular momentum and the angular momentum of the planetary rotation. We suspect that the planetary atmosphere may participate in an exchange of momentum between these two reservoirs. Nontrivial changes in the circulation of the atmosphere are likely to occur, as the atmospheric system gains and loses angular momentum, during this exchange. We derive a coupling expression linking orbital and rotational motions that produces an acceleration field varying with position and with time on and within a subject body. The spatially and temporally varying accelerations may interfere constructively or destructively with large-scale flows of geophysical fluids that are established and maintained by other means. This physical hypothesis predicts cycles of intensification and relaxation of circulatory flows of atmospheres on seasonal and longer timescales that are largely independent of solar forcing. The predictions of this hypothesis may be tested through numerical modeling. Examples from investigations of the atmospheric circulation of Mars are provided to illustrate qualitative features and quantitative aspects of the coupling mechanism proposed.

Phosphatidylinositol 3-kinase inhibition restores Ca2+ release defects and prolongs survival in myotubularin-deficient mice

PubMed Central

Kutchukian, Candice; Lo Scrudato, Mirella; Tourneur, Yves; Poulard, Karine; Vignaud, Alban; Berthier, Christine; Allard, Bruno; Lawlor, Michael W.; Buj-Bello, Ana; Jacquemond, Vincent

2016-01-01

Mutations in the gene encoding the phosphoinositide 3-phosphatase myotubularin (MTM1) are responsible for a pediatric disease of skeletal muscle named myotubular myopathy (XLMTM). Muscle fibers from MTM1-deficient mice present defects in excitation–contraction (EC) coupling likely responsible for the disease-associated fatal muscle weakness. However, the mechanism leading to EC coupling failure remains unclear. During normal skeletal muscle EC coupling, transverse (t) tubule depolarization triggers sarcoplasmic reticulum (SR) Ca2+ release through ryanodine receptor channels gated by conformational coupling with the t-tubule voltage-sensing dihydropyridine receptors. We report that MTM1 deficiency is associated with a 60% depression of global SR Ca2+ release over the full range of voltage sensitivity of EC coupling. SR Ca2+ release in the diseased fibers is also slower than in normal fibers, or delayed following voltage activation, consistent with the contribution of Ca2+-gated ryanodine receptors to EC coupling. In addition, we found that SR Ca2+ release is spatially heterogeneous within myotubularin-deficient muscle fibers, with focally defective areas recapitulating the global alterations. Importantly, we found that pharmacological inhibition of phosphatidylinositol 3-kinase (PtdIns 3-kinase) activity rescues the Ca2+ release defects in isolated muscle fibers and increases the lifespan and mobility of XLMTM mice, providing proof of concept for the use of PtdIns 3-kinase inhibitors in myotubular myopathy and suggesting that unbalanced PtdIns 3-kinase activity plays a critical role in the pathological process. PMID:27911767

Recent trends in energy flows through the Arctic climate system

NASA Astrophysics Data System (ADS)

Mayer, Michael; Haimberger, Leo

2016-04-01

While Arctic climate change can be diagnosed in many parameters, a comprehensive assessment of long-term changes and low frequency variability in the coupled Arctic energy budget still remains challenging due to the complex physical processes involved and the lack of observations. Here we draw on strongly improved observational capabilities of the past 15 years and employ observed radiative fluxes from CERES along with state-of-the-art atmospheric as well as coupled ocean-ice reanalyses to explore recent changes in energy flows through the Arctic climate system. Various estimates of ice volume and ocean heat content trends imply that the energy imbalance of the Arctic climate system was >1 Wm-2 during the 2000-2015 period, where most of the extra heat warmed the ocean and a comparatively small fraction was used to melt sea ice. The energy imbalance was partly fed by enhanced oceanic heat transports into the Arctic, especially in the mid 2000s. Seasonal trends of net radiation show a very clear signal of the ice-albedo feedback. Stronger radiative energy input during summer means increased seasonal oceanic heat uptake and accelerated sea ice melt. In return, lower minimum sea ice extent and higher SSTs lead to enhanced heat release from the ocean during fall season. These results are consistent with modeling studies finding an enhancement of the annual cycle of surface energy exchanges in a warming Arctic. Moreover, stronger heat fluxes from the ocean to the atmosphere in fall tend to warm the arctic boundary layer and reduce meridional temperature gradients, thereby reducing atmospheric energy transports into the polar cap. Although the observed results are a robust finding, extended high-quality datasets are needed to reliably separate trends from low frequency variability.

Arctic sea-ice variability and its implication to the path of pollutants under a changing climate

NASA Astrophysics Data System (ADS)

Castro-Morales, K.; Gerdes, R.; Riemann-Campe, K.; Köberle, C.; Losch, M.

2012-04-01

The increasing concentration of pollutants from anthropogenic origin in the Arctic atmosphere, water, sediments and biota has been evident during the last decade. The sea-ice is an important vehicle for pollutants in the Arctic Ocean. Pollutants are taken up by precipitation and dry atmospheric deposition over the snow and ice cover during winter and released to the ocean during melting. Recent changes in the sea-ice cover of the Arctic Ocean affect the fresh water balance and the oceanic circulation, and with it, the fate of pollutants in the system. The Arctic Ocean is characterized by complex dynamics and strong stratification. Thus, to evaluate the current and future changes in the Arctic circulation high-resolution models are needed. As part of the EU FP7 project ArcRisk (under the scope of the IPY), we use a high resolution regional sea-ice-ocean coupled model covering the Arctic Ocean and the subpolar North Atlantic based on the Massachusetts Institute of Technology - circulation model (MITgcm). Under realistic atmospheric forcing we obtain hindcast results of circulation patterns for the period 1990 - 2010 for validation of the model. We evaluate possible consequences on the pathways and transport of contaminants by downscaling future climate scenario runs available in the coupled model intercomparison project (CMIP3) for the following fifty years. Particular interest is set in the Barents Sea. In this shallow region strong river runoff, sea-ice delivered from the interior of the Arctic Ocean and warm waters from the North Atlantic current are main sources of contaminants. Under a changing climate, a higher input of contaminants delivered to surface waters is expected, remaining in the interior of the Arctic Ocean in a strongly stratified water column remaining.

Lunar volcanism produced a transient atmosphere around the ancient Moon

NASA Astrophysics Data System (ADS)

Needham, Debra H.; Kring, David A.

2017-11-01

Studies of the lunar atmosphere have shown it to be a stable, low-density surface boundary exosphere for the last 3 billion years. However, substantial volcanic activity on the Moon prior to 3 Ga may have released sufficient volatiles to form a transient, more prominent atmosphere. Here, we calculate the volume of mare basalt emplaced as a function of time, then estimate the corresponding production of volatiles released during the mare basalt-forming eruptions. Results indicate that during peak mare emplacement and volatile release ∼3.5 Ga, the maximum atmospheric pressure at the lunar surface could have reached ∼1 kPa, or ∼1.5 times higher than Mars' current atmospheric surface pressure. This lunar atmosphere may have taken ∼70 million years to fully dissipate. Most of the volatiles released by mare basalts would have been lost to space, but some may have been sequestered in permanently shadowed regions on the lunar surface. If only 0.1% of the mare water vented during these eruptions remains in the polar regions of the Moon, volcanically-derived volatiles could account for all hydrogen deposits - suspected to be water - currently observed in the Moon's permanently shadowed regions. Future missions to such locations may encounter evidence of not only asteroidal, cometary, and solar wind-derived volatiles, but also volatiles vented from the interior of the Moon.

Using Atmospheric Dispersion Theory to Inform the Design of a Short-lived Radioactive Particle Release Experiment

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rishel, Jeremy P.; Keillor, Martin E.; Arrigo, Leah M.

2016-01-01

Atmospheric dispersion theory can be used to predict ground deposition of particulates downwind of a radionuclide release. This paper utilizes standard formulations found in Gaussian plume models to inform the design of an experimental release of short-lived radioactive particles into the atmosphere. Specifically, a source depletion algorithm is used to determine the optimum particle size and release height that maximizes the near-field deposition while minimizing the both the required source activity and the fraction of activity lost to long-distance transport. The purpose of the release is to provide a realistic deposition pattern that might be observed downwind of a small-scalemore » vent from an underground nuclear explosion. The deposition field will be used, in part, to investigate several techniques of gamma radiation survey and spectrometry that could be utilized by an On-Site Inspection team under the verification regime of the Comprehensive Nuclear-Test-Ban Treaty.« less

A System of Conservative Regridding for Ice-Atmosphere Coupling in a General Circulation Model (GCM)

NASA Technical Reports Server (NTRS)

Fischer, R.; Nowicki, S.; Kelley, M.; Schmidt, G. A.

2014-01-01

The method of elevation classes, in which the ice surface model is run at multiple elevations within each grid cell, has proven to be a useful way for a low-resolution atmosphere inside a general circulation model (GCM) to produce high-resolution downscaled surface mass balance fields for use in one-way studies coupling atmospheres and ice flow models. Past uses of elevation classes have failed to conserve mass and energy because the transformation used to regrid to the atmosphere was inconsistent with the transformation used to downscale to the ice model. This would cause problems for two-way coupling. A strategy that resolves this conservation issue has been designed and is presented here. The approach identifies three grids between which data must be regridded and five transformations between those grids required by a typical coupled atmosphere-ice flow model. This paper develops a theoretical framework for the problem and shows how each of these transformations may be achieved in a consistent, conservative manner. These transformations are implemented in Glint2, a library used to couple atmosphere models with ice models. Source code and documentation are available for download. Confounding real-world issues are discussed, including the use of projections for ice modeling, how to handle dynamically changing ice geometry, and modifications required for finite element ice models.

Methane ebullition fluxes from northern peatlands: initial observations from four sites of contrasting vegetation type in Caribou Bog, ME

NASA Astrophysics Data System (ADS)

Slater, L. D.; Comas, X.; Mumford, K. G.; Reeve, A. S.; Varner, R. K.; Chen, X.; Wright, W.; Wright, J.; Molnar, I. L.; Krol, M.

2017-12-01

The contribution of peatlands to the atmospheric CH4 burden remains unclear in large part due to incomplete understanding of the ebullition pathway. Oxidation of dissolved methane reduces the release of methane by diffusion, but the transit time of bubbles released via ebullition is too short for extensive oxidation to occur, i.e. ebullition releases increase the greenhouse gas potential of peatlands. We are working to couple innovative strategies for ebullition monitoring with a physical model describing gas transport in terms of the mechanical properties of the peat. This integration of measurement and modeling will permit a fundamental step forward towards a more quantitative understanding of CH4 ebullition from peatlands. Sampling and sensor installation have been performed in Caribou Bog, a multi-unit peatland located in Maine (USA) where an extensive database accounting for a decade of research is already available from previous work examining methane dynamics. Multi-depth gas trap and moisture probe arrays have been installed at four sites selected based on contrasting vegetation type and peat basin depth determined from extensive ground penetrating radar surveys. Hydraulic head measurements have also been acquired on multi-level piezometers designed to capture transient signals associated with gas transport. Cores and initial field observations acquired in summer 2017 confirm that the physical properties of the peat vary markedly between the sites and influence gas storage and release. An existing ebullition model describing gas bubble expansion is being coupled with an invasion percolation approach to describe the transport of CH4 between multiple peat layers by both diffusion in the pore water and ebullition between layers. Although the proposed model does not explicitly incorporate the geomechanical properties of peat, model predictions for maximum gas contents are being compared with key measurable geomechanical properties (including measured capillary drainage curves for peat) that may control ebullition.

Total mercury released to the environment by human activities

DOE Office of Scientific and Technical Information (OSTI.GOV)

Streets, David G.; Horowitz, Hannah M.; Jacob, Daniel J.

Here, we estimate that a cumulative total of 1.5 (1.0–2.8) Tg (teragrams, or million tonnes) of mercury (Hg) have been released by human activities up to 2010, 73% of which was released after 1850. Of this liberated Hg, 470 Gg (gigagrams, or thousand tonnes) was emitted directly into the air, and 74% of the air emissions were elemental Hg. Cumulatively, about 1.1 Tg were released to land and water bodies. Though annual releases of Hg have been relatively stable since 1880 at 8 ± 2 Gg, except for wartime, the distributions of those releases among source types, world regions, andmore » environmental media have changed dramatically. Production of Hg accounts for 27% of cumulative Hg releases to the environment, followed by silver mining (24%) and chemicals manufacturing (12%). North America (30%), Europe (27%), and Asia (16%) have experienced the largest releases. Biogeochemical modeling shows a 3.2-fold increase in the atmospheric burden relative to 1850 and a contemporary atmospheric reservoir of 4570 Mg, both of which agree well with observational constraints. We find that approximately 40% (390 Gg) of the Hg discarded to land and water must be sequestered at contaminated sites to maintain consistency with recent declines in atmospheric Hg concentrations.« less

Total mercury released to the environment by human activities

DOE PAGES

Streets, David G.; Horowitz, Hannah M.; Jacob, Daniel J.; ...

2017-04-27

Here, we estimate that a cumulative total of 1.5 (1.0–2.8) Tg (teragrams, or million tonnes) of mercury (Hg) have been released by human activities up to 2010, 73% of which was released after 1850. Of this liberated Hg, 470 Gg (gigagrams, or thousand tonnes) was emitted directly into the air, and 74% of the air emissions were elemental Hg. Cumulatively, about 1.1 Tg were released to land and water bodies. Though annual releases of Hg have been relatively stable since 1880 at 8 ± 2 Gg, except for wartime, the distributions of those releases among source types, world regions, andmore » environmental media have changed dramatically. Production of Hg accounts for 27% of cumulative Hg releases to the environment, followed by silver mining (24%) and chemicals manufacturing (12%). North America (30%), Europe (27%), and Asia (16%) have experienced the largest releases. Biogeochemical modeling shows a 3.2-fold increase in the atmospheric burden relative to 1850 and a contemporary atmospheric reservoir of 4570 Mg, both of which agree well with observational constraints. We find that approximately 40% (390 Gg) of the Hg discarded to land and water must be sequestered at contaminated sites to maintain consistency with recent declines in atmospheric Hg concentrations.« less

Investigation of hurricane Ivan using the coupled ocean-atmosphere-wave-sediment transport (COAWST) model

USGS Publications Warehouse

Zambon, Joseph B.; He, Ruoying; Warner, John C.

2014-01-01

The coupled ocean–atmosphere–wave–sediment transport (COAWST) model is used to hindcast Hurricane Ivan (2004), an extremely intense tropical cyclone (TC) translating through the Gulf of Mexico. Sensitivity experiments with increasing complexity in ocean–atmosphere–wave coupled exchange processes are performed to assess the impacts of coupling on the predictions of the atmosphere, ocean, and wave environments during the occurrence of a TC. Modest improvement in track but significant improvement in intensity are found when using the fully atmosphere–ocean-wave coupled configuration versus uncoupled (e.g., standalone atmosphere, ocean, or wave) model simulations. Surface wave fields generated in the fully coupled configuration also demonstrates good agreement with in situ buoy measurements. Coupled and uncoupled model-simulated sea surface temperature (SST) fields are compared with both in situ and remote observations. Detailed heat budget analysis reveals that the mixed layer temperature cooling in the deep ocean (on the shelf) is caused primarily by advection (equally by advection and diffusion).

Preface of the special issue: "Vertical coupling in the atmosphere-ionosphere system: Recent progress"

NASA Astrophysics Data System (ADS)

2018-06-01

This special issue of the Journal of Atmospheric and Solar-Terrestrial Physics comprises papers dealing with investigation of the coupling phenomena in the neutral Atmosphere-Ionosphere System of the Earth. The core of the special issue is formed by the recent results presented during the 6th IAGA/ICMA/SCOSTEP Workshop on the Vertical Coupling in the Neutral Atmosphere-Ionosphere System held in Taipei, Taiwan, July 2016. Workshops are organized with a substantial support of the scientific international bodies, such as the International Association of Geomagnetism and Aeronomy (IAGA), International Commission for the Middle Atmosphere (ICMA) and Committee on Solar-Terrestrial Physics (SCOSTEP). The special issue includes also recent results of other members of the aeronomic research community. Hence it represents the state-of-art knowledge in the associated research fields.

Medicanes in an ocean-atmosphere coupled regional climate model

NASA Astrophysics Data System (ADS)

Akhtar, N.; Brauch, J.; Dobler, A.; Béranger, K.; Ahrens, B.

2014-03-01

So-called medicanes (Mediterranean hurricanes) are meso-scale, marine, and warm-core Mediterranean cyclones that exhibit some similarities to tropical cyclones. The strong cyclonic winds associated with medicanes threaten the highly populated coastal areas around the Mediterranean basin. To reduce the risk of casualties and overall negative impacts, it is important to improve the understanding of medicanes with the use of numerical models. In this study, we employ an atmospheric limited-area model (COSMO-CLM) coupled with a one-dimensional ocean model (1-D NEMO-MED12) to simulate medicanes. The aim of this study is to assess the robustness of the coupled model in simulating these extreme events. For this purpose, 11 historical medicane events are simulated using the atmosphere-only model, COSMO-CLM, and coupled model, with different setups (horizontal atmospheric grid-spacings of 0.44°, 0.22°, and 0.08°; with/without spectral nudging, and an ocean grid-spacing of 1/12°). The results show that at high-resolution, the coupled model is able to not only simulate most of medicane events but also improve the track length, core temperature, and wind speed of simulated medicanes compared to the atmosphere-only simulations. The results suggest that the coupled model is more proficient for systemic and detailed studies of historical medicane events, and that this model can be an effective tool for future projections.

Medicanes in an ocean-atmosphere coupled regional climate model

NASA Astrophysics Data System (ADS)

Akhtar, N.; Brauch, J.; Dobler, A.; Béranger, K.; Ahrens, B.

2014-08-01

So-called medicanes (Mediterranean hurricanes) are meso-scale, marine, and warm-core Mediterranean cyclones that exhibit some similarities to tropical cyclones. The strong cyclonic winds associated with medicanes threaten the highly populated coastal areas around the Mediterranean basin. To reduce the risk of casualties and overall negative impacts, it is important to improve the understanding of medicanes with the use of numerical models. In this study, we employ an atmospheric limited-area model (COSMO-CLM) coupled with a one-dimensional ocean model (1-D NEMO-MED12) to simulate medicanes. The aim of this study is to assess the robustness of the coupled model in simulating these extreme events. For this purpose, 11 historical medicane events are simulated using the atmosphere-only model, COSMO-CLM, and coupled model, with different setups (horizontal atmospheric grid spacings of 0.44, 0.22, and 0.08°; with/without spectral nudging, and an ocean grid spacing of 1/12°). The results show that at high resolution, the coupled model is able to not only simulate most of medicane events but also improve the track length, core temperature, and wind speed of simulated medicanes compared to the atmosphere-only simulations. The results suggest that the coupled model is more proficient for systemic and detailed studies of historical medicane events, and that this model can be an effective tool for future projections.

Effects of Atmospheric Conditions and the Land/Atmospheric Interface on Transport of Chemical Vapors from Subsurface Sources

NASA Astrophysics Data System (ADS)

Rice, A. K.; Smits, K. M.; Cihan, A.; Howington, S. E.; Illangasekare, T. H.

2013-12-01

Understanding the movement of chemical vapors and gas through variably saturated soil subjected to atmospheric thermal and mass flux boundary conditions at the land/atmospheric interface is important to many applications, including landmine detection, methane leakage during natural gas production from shale and CO2 leakage from deep geologic storage. New, advanced technologies exist to sense chemical signatures and gas leakage at the land/atmosphere interface, but interpretation of sensor signals remains a challenge. Chemical vapors are subject to numerous interactions while migrating through the soil environment, masking source conditions. The process governing movement of gases through porous media is often assumed to be Fickian diffusion through the air phase with minimal quantification of other processes, such as convective gas flow and temporal or spatial variation in soil moisture. Vapor migration is affected by atmospheric conditions (e.g. humidity, temperature, wind velocity), soil thermal and hydraulic properties and contaminant properties, all of which are physically and thermodynamically coupled. The complex coupling of two drastically different flow regimes in the subsurface and atmosphere is commonly ignored in modeling efforts, or simplifying assumptions are made to treat the systems as de-coupled. Experimental data under controlled laboratory settings are lacking to refine the theory for proper coupling and complex treatment of vapor migration through porous media in conversation with atmospheric flow and climate variations. Improving fundamental understanding and accurate quantification of these processes is not feasible in field settings due to lack of controlled initial and boundary conditions and inability to fully characterize the subsurface at all relevant scales. The goal of this work is to understand the influence of changes in atmospheric conditions to transport of vapors through variably saturated soil. We have developed a tank apparatus with a network of soil and atmospheric sensors and a head space for air flow to simulate the atmospheric boundary layer. Experiments were performed under varying temperature values at the soil surface bounded by the atmospheric boundary layer. The model of Smits et al. [2011], accounting for non-equilibrium phase change and coupled heat, water vapor and liquid water flux through soil, was amended to include organic vapor in the gas phase and migration mechanisms often overlooked in models (thermal and Knudsen diffusion, density driven advection). Experimental results show increased vapor mass flux across the soil/atmospheric interface due to heat applied from the atmosphere and coupling of heat and mass transfer in the shallow subsurface for both steady and diurnal temperature patterns. Comparison of model results to experimental data shows dynamic interactions between transport in porous media and boundary conditions. Results demonstrate the value of considering interactions of the atmosphere and subsurface to better understand chemical gas transport through unsaturated soils and the land/atmospheric interface.

Upper Atmosphere Research Satellite (UARS): A program to study global ozone change

NASA Technical Reports Server (NTRS)

1991-01-01

A general overview of NASA's Upper Atmosphere Research Satellite (UARS) program is presented in a broad based informational publication. The UARS will be responsible for carrying out the first systematic, comprehensive study of the stratosphere and will furnish important new data on the mesosphere and thermosphere. The UARS mission objectives are to provide an increased understanding of energy input into the upper atmosphere; global photochemistry of the upper atmosphere; dynamics of the upper atmosphere; coupling among these processes; and coupling between the upper and lower atmosphere. These mission objectives are briefly described along with the UARS on-board instrumentation and related data management systems.

Effects of explicit convection on global land-atmosphere coupling in the superparameterized CAM

DOE PAGES

Sun, Jian; Pritchard, Michael S.

2016-07-25

Here, conventional global climate models are prone to producing unrealistic land-atmosphere coupling signals. Cumulus and convection parameterizations are natural culprits but the effect of bypassing them with explicitly resolved convection on global land-atmosphere coupling dynamics has not been explored systematically. We apply a suite of modern land-atmosphere coupling diagnostics to isolate the effect of cloud Superparameterization in the Community Atmosphere Model (SPCAM) v3.5, focusing on both the terrestrial segment (i.e., soil moisture and surface turbulent fluxes interaction) and atmospheric segment (i.e., surface turbulent fluxes and precipitation interaction) in the water pathway of the landatmosphere feedback loop. At daily timescales, SPCAMmore » produces stronger uncoupled terrestrial signals (negative sign) over tropical rainforests in wet seasons, reduces the terrestrial coupling strength in the Central Great Plain in American, and reverses the coupling sign (from negative to positive) over India in the boreal summer season—all favorable improvements relative to reanalysis-forced land modeling. Analysis of the triggering feedback strength (TFS) and amplification feedback strength (AFS) shows that SPCAM favorably reproduces the observed geographic patterns of these indices over North America, with the probability of afternoon precipitation enhanced by high evaporative fraction along the eastern United States and Mexico, while conventional CAM does not capture this signal. We introduce a new diagnostic called the Planetary Boundary Layer (PBL) Feedback Strength (PFS), which reveals that SPCAM exhibits a tight connection between the responses of the lifting condensation level, the PBL height, and the rainfall triggering to surface turbulent fluxes; a triggering disconnect is found in CAM.« less

Effects of explicit convection on global land-atmosphere coupling in the superparameterized CAM

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sun, Jian; Pritchard, Michael S.

Here, conventional global climate models are prone to producing unrealistic land-atmosphere coupling signals. Cumulus and convection parameterizations are natural culprits but the effect of bypassing them with explicitly resolved convection on global land-atmosphere coupling dynamics has not been explored systematically. We apply a suite of modern land-atmosphere coupling diagnostics to isolate the effect of cloud Superparameterization in the Community Atmosphere Model (SPCAM) v3.5, focusing on both the terrestrial segment (i.e., soil moisture and surface turbulent fluxes interaction) and atmospheric segment (i.e., surface turbulent fluxes and precipitation interaction) in the water pathway of the landatmosphere feedback loop. At daily timescales, SPCAMmore » produces stronger uncoupled terrestrial signals (negative sign) over tropical rainforests in wet seasons, reduces the terrestrial coupling strength in the Central Great Plain in American, and reverses the coupling sign (from negative to positive) over India in the boreal summer season—all favorable improvements relative to reanalysis-forced land modeling. Analysis of the triggering feedback strength (TFS) and amplification feedback strength (AFS) shows that SPCAM favorably reproduces the observed geographic patterns of these indices over North America, with the probability of afternoon precipitation enhanced by high evaporative fraction along the eastern United States and Mexico, while conventional CAM does not capture this signal. We introduce a new diagnostic called the Planetary Boundary Layer (PBL) Feedback Strength (PFS), which reveals that SPCAM exhibits a tight connection between the responses of the lifting condensation level, the PBL height, and the rainfall triggering to surface turbulent fluxes; a triggering disconnect is found in CAM.« less

Development and applications of a Coupled-Ocean-Atmosphere-Wave-Sediment Transport (COAWST) Modeling System

NASA Astrophysics Data System (ADS)

Warner, J. C.; Armstrong, B. N.; He, R.; Zambon, J. B.; Olabarrieta, M.; Voulgaris, G.; Kumar, N.; Haas, K. A.

2012-12-01

Understanding processes responsible for coastal change is important for managing both our natural and economic coastal resources. Coastal processes respond from both local scale and larger regional scale forcings. Understanding these processes can lead to significant insight into how the coastal zone evolves. Storms are one of the primary driving forces causing coastal change from a coupling of wave and wind driven flows. Here we utilize a numerical modeling approach to investigate these dynamics of coastal storm impacts. We use the Coupled Ocean - Atmosphere - Wave - Sediment Transport (COAWST) Modeling System that utilizes the Model Coupling Toolkit to exchange prognostic variables between the ocean model ROMS, atmosphere model WRF, wave model SWAN, and the Community Sediment Transport Modeling System (CSTMS) sediment routines. The models exchange fields of sea-surface temperature, ocean currents, water levels, bathymetry, wave heights, lengths, periods, bottom orbital velocities, and atmospheric surface heat and momentum fluxes, atmospheric pressure, precipitation, and evaporation. Data fields are exchanged using regridded flux conservative sparse matrix interpolation weights computed from the SCRIP spherical coordinate remapping interpolation package. We describe the modeling components and the model field exchange methods. As part of the system, the wave and ocean models run with cascading, refined, spatial grids to provide increased resolution, scaling down to resolve nearshore wave driven flows simulated by the vortex force formulation, all within selected regions of a larger, coarser-scale coastal modeling system. The ocean and wave models are driven by the atmospheric component, which is affected by wave dependent ocean-surface roughness and sea surface temperature which modify the heat and momentum fluxes at the ocean-atmosphere interface. We describe the application of the modeling system to several regions of multi-scale complexity to identify the significance of larger scale forcing cascading down to smaller scales and to investigate the interactions of the coupled system with increasing degree of model-model interactions. Three examples include the impact of Hurricane Ivan in 2004 in the Gulf of Mexico, Hurricane Ida in 2009 that evolved into a tropical storm on the US East coast, and passage of strong cold fronts across the US southeast. Results identify that hurricane intensity is extremely sensitive to sea-surface temperature, with a reduction in intensity when the atmosphere is coupled to the ocean model due to rapid cooling of the ocean from the surface through the mixed layer. Coupling of the ocean to the atmosphere also results in decreased boundary layer stress and coupling of the waves to the atmosphere results in increased sea-surface stress. Wave results are sensitive to both ocean and atmospheric coupling due to wave-current interactions with the ocean and wave-growth from the atmospheric wind stress. Sediment resuspension at regional scale during the hurricane is controlled by shelf width and wave propagation during hurricane approach. Results from simulation of passage of cold fronts suggest that synoptic meteorological systems can strongly impact surf zone and inner shelf response, therefore act as a strong driver for long term littoral sediment transport. We will also present some of the challenges faced to develop the modeling system.

Effects of air-sea coupling over the North Sea and the Baltic Sea on simulated summer precipitation over Central Europe

NASA Astrophysics Data System (ADS)

Ho-Hagemann, Ha Thi Minh; Gröger, Matthias; Rockel, Burkhardt; Zahn, Matthias; Geyer, Beate; Meier, H. E. Markus

2017-12-01

This study introduces a new approach to investigate the potential effects of air-sea coupling on simulated precipitation inland over Central Europe. We present an inter-comparison of two regional climate models (RCMs), namely, the COSMO-CLM (hereafter CCLM) and RCA4 models, which are configured for the EURO-CORDEX domain in the coupled and atmosphere-only modes. Two versions of the CCLM model, namely, 4.8 and 5.0, join the inter-comparison being almost two different models while providing pronouncedly different summer precipitation simulations because of many changes in the dynamics and physics of CCLM in version 5.0. The coupling effect on the prominent summer dry bias over Central Europe is analysed using seasonal (JJA) mean statistics for the 30-year period from 1979 to 2009, with a focus on extreme precipitation under specific weather regimes. The weather regimes are compared between the coupled and uncoupled simulations to better understand the mechanism of the coupling effects. The comparisons of the coupled systems with the atmosphere-only models show that coupling clearly reduces the dry bias over Central Europe for CCLM 4.8, which has a large dry summer bias, but not for CCLM 5.0 and RCA4, which have smaller dry biases. This result implies that if the atmosphere-only model already yields reasonable summer precipitation over Central Europe, not much room for improvement exists that can be caused by the air-sea coupling over the North Sea and the Baltic Sea. However, if the atmosphere-only model shows a pronounced summer dry bias because of a lack of moisture transport from the seas into the region, the considered coupling may create an improved simulation of summer precipitation over Central Europe, such as for CCLM 4.8. For the latter, the benefit of coupling varies over the considered timescales. The precipitation simulations that are generated by the coupled system COSTRICE 4.8 and the atmosphere-only CCLM 4.8 are mostly identical for the summer mean. However, the COSTRICE simulations are generally more accurate than the atmosphere-only CCLM simulations if extreme precipitation is considered, particularly under Northerly Circulation conditions, in which the airflow from the North Atlantic Ocean passes the North Sea in the coupling domain. The air-sea feedback (e.g., wind, evaporation and sea surface temperature) and land-sea interactions are better reproduced with the COSTRICE model system than the atmosphere-only CCLM and lead to an improved simulation of large-scale moisture convergence from the sea to land and, consequently, increased heavy precipitation over Central Europe.

Studying urban land-atmospheric interactions by coupling an urban canopy model with a single column atmospheric models

NASA Astrophysics Data System (ADS)

Song, J.; Wang, Z.

2013-12-01

Studying urban land-atmospheric interactions by coupling an urban canopy model with a single column atmospheric models Jiyun Song and Zhi-Hua Wang School of Sustainable Engineering and the Built Environment, Arizona State University, PO Box 875306, Tempe, AZ 85287-5306 Landuse landcover changes in urban area will modify surface energy budgets, turbulent fluxes as well as dynamic and thermodynamic structures of the overlying atmospheric boundary layer (ABL). In order to study urban land-atmospheric interactions, we coupled a single column atmospheric model (SCM) to a cutting-edge single layer urban canopy model (SLUCM). Modification of surface parameters such as the fraction of vegetation and engineered pavements, thermal properties of building and pavement materials, and geometrical features of street canyon, etc. in SLUCM dictates the evolution of surface balance of energy, water and momentum. The land surface states then provide lower boundary conditions to the overlying atmosphere, which in turn modulates the modification of ABL structure as well as vertical profiles of temperature, humidity, wind speed and tracer gases. The coupled SLUCM-SCM model is tested against field measurements of surface layer fluxes as well as profiles of temperature and humidity in the mixed layer under convective conditions. After model test, SLUCM-SCM is used to simulate the effect of changing urban land surface conditions on the evolution of ABL structure and dynamics. Simulation results show that despite the prescribed atmospheric forcing, land surface states impose significant impact on the physics of the overlying vertical atmospheric layer. Overall, this numerical framework provides a useful standalone modeling tool to assess the impacts of urban land surface conditions on the local hydrometeorology through land-atmospheric interactions. It also has potentially far-reaching implications to urban ecohydrological services for cities under future expansion and climate challenges.

The kinetics of aerosol particle formation and removal in NPP severe accidents

NASA Astrophysics Data System (ADS)

Zatevakhin, Mikhail A.; Arefiev, Valentin K.; Semashko, Sergey E.; Dolganov, Rostislav A.

2016-06-01

Severe Nuclear Power Plant (NPP) accidents are accompanied by release of a massive amount of energy, radioactive products and hydrogen into the atmosphere of the NPP containment. A valid estimation of consequences of such accidents can only be carried out through the use of the integrated codes comprising a description of the basic processes which determine the consequences. A brief description of a coupled aerosol and thermal-hydraulic code to be used for the calculation of the aerosol kinetics within the NPP containment in case of a severe accident is given. The code comprises a KIN aerosol unit integrated into the KUPOL-M thermal-hydraulic code. Some features of aerosol behavior in severe NPP accidents are briefly described.

The kinetics of aerosol particle formation and removal in NPP severe accidents

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zatevakhin, Mikhail A.; Arefiev, Valentin K.; Semashko, Sergey E.

2016-06-08

Severe Nuclear Power Plant (NPP) accidents are accompanied by release of a massive amount of energy, radioactive products and hydrogen into the atmosphere of the NPP containment. A valid estimation of consequences of such accidents can only be carried out through the use of the integrated codes comprising a description of the basic processes which determine the consequences. A brief description of a coupled aerosol and thermal–hydraulic code to be used for the calculation of the aerosol kinetics within the NPP containment in case of a severe accident is given. The code comprises a KIN aerosol unit integrated into themore » KUPOL-M thermal–hydraulic code. Some features of aerosol behavior in severe NPP accidents are briefly described.« less

Decreased atmospheric sulfur deposition across the southeastern U.S.: When will watersheds release stored sulfate?

USGS Publications Warehouse

Rice, Karen C.; Scanlon, Todd M.; Lynch, Jason A.; Cosby, Bernard J.

2014-01-01

Emissions of sulfur dioxide (SO2) to the atmosphere lead to atmospheric deposition of sulfate (SO42-), which is the dominant strong acid anion causing acidification of surface waters and soils in the eastern United States (U.S.). Since passage of the Clean Air Act and its Amendments, atmospheric deposition of SO2 in this region has declined by over 80%, but few corresponding decreases in stream-water SO42- concentrations have been observed in unglaciated watersheds. We calculated SO42- mass balances for 27 forested, unglaciated watersheds from Pennsylvania to Georgia, by using total atmospheric deposition (wet plus dry) as input. Many of these watersheds still retain SO42-, unlike their counterparts in the northeastern U.S. and southern Canada. Our analysis showed that many of these watersheds should convert from retaining to releasing SO42- over the next two decades. The specific years when the watersheds crossover from retaining to releasing SO42- correspond to a general geographical pattern of later net watershed release from north to south. The single most important variable that explained the crossover year was the runoff ratio, defined as the ratio of annual mean stream discharge to precipitation. Percent clay content and mean soil depth were secondary factors in predicting crossover year. The conversion of watersheds from net SO42- retention to release anticipates more widespread reductions in stream-water SO42- concentrations in this region.

Decreased atmospheric sulfur deposition across the Southeastern U.S.: when will watersheds release stored sulfate?

PubMed

Rice, Karen C; Scanlon, Todd M; Lynch, Jason A; Cosby, Bernard J

2014-09-02

Emissions of sulfur dioxide (SO2) to the atmosphere lead to atmospheric deposition of sulfate (SO4(2-)), which is the dominant strong acid anion causing acidification of surface waters and soils in the eastern United States. Since passage of the Clean Air Act and its Amendments, atmospheric deposition of SO2 in this region has declined by over 80%, but few corresponding decreases in streamwater SO4(2-) concentrations have been observed in unglaciated watersheds. We calculated SO4(2-) mass balances for 27 forested, unglaciated watersheds from Pennsylvania to Georgia, by using total atmospheric deposition (wet plus dry) as input. Many of these watersheds still retain SO4(2-), unlike their counterparts in the northeastern U.S. and southern Canada. Our analysis showed that many of these watersheds should convert from retaining to releasing SO4(2-) over the next two decades. The specific years when the watersheds crossover from retaining to releasing SO4(2-) correspond to a general geographical pattern of later net watershed release from north to south. The single most important variable that explained the crossover year was the runoff ratio, defined as the ratio of annual mean stream discharge to precipitation. Percent clay content and mean soil depth were secondary factors in predicting crossover year. The conversion of watersheds from net SO4(2-) retention to release anticipates more widespread reductions in streamwater SO4(2-) concentrations in this region.

DSCOVR EPIC L2 Atmospheric Correction (MAIAC) Data Release Announcement

Atmospheric Science Data Center

2018-06-22

... several atmospheric quantities including cloud mask and aerosol optical depth (AOD) required for atmospheric correction. The parameters ... is a useful complementary dataset to MODIS and VIIRS global aerosol products.   Information about the DSCOVR EPIC Atmospheric ...

BIOGENIC HYDROCARBONS IN THE ATMOSPHERIC BOUNDARY LAYER: A REVIEW

EPA Science Inventory

Nonmethane hydrocarbons are ubiquitous trace atmospheric constituents yet they control the oxidation capacity of the atmosphere. Both anthropogenic and biogenic processes contribute to the release of hydrocarbons to the atmosphere. In this manuscript, the state of the science ...

The Double ITCZ Syndrome in GCMs: A Coupled Problem among Convection, Atmospheric and Ocean Circulations

NASA Astrophysics Data System (ADS)

Zhang, G. J.; Song, X.

2017-12-01

The double ITCZ bias has been a long-standing problem in coupled atmosphere-ocean models. A previous study indicates that uncertainty in the projection of global warming due to doubling of CO2 is closely related to the double ITCZ biases in global climate models. Thus, reducing the double ITCZ biases is not only important to getting the current climate features right, but also important to narrowing the uncertainty in future climate projection. In this work, we will first review the possible factors contributing to the ITCZ problem. Then, we will focus on atmospheric convection, presenting recent progress in alleviating the double ITCZ problem and its sensitivity to details of convective parameterization, including trigger conditions for convection onset, convective memory, entrainment rate, updraft model and closure in the NCAR CESM1. These changes together can result in dramatic improvements in the simulation of ITCZ. Results based on both atmospheric only and coupled simulations with incremental changes of convection scheme will be shown to demonstrate the roles of convection parameterization and coupled interaction between convection, atmospheric circulation and ocean circulation in the simulation of ITCZ.

40 CFR 68.165 - Offsite consequence analysis.

Code of Federal Regulations, 2013 CFR

2013-07-01

... (CONTINUED) CHEMICAL ACCIDENT PREVENTION PROVISIONS Risk Management Plan § 68.165 Offsite consequence... released in pounds; (7) Release rate; (8) Release duration; (9) Wind speed and atmospheric stability class...

40 CFR 68.165 - Offsite consequence analysis.

Code of Federal Regulations, 2012 CFR

2012-07-01

... (CONTINUED) CHEMICAL ACCIDENT PREVENTION PROVISIONS Risk Management Plan § 68.165 Offsite consequence... released in pounds; (7) Release rate; (8) Release duration; (9) Wind speed and atmospheric stability class...

40 CFR 68.165 - Offsite consequence analysis.

Code of Federal Regulations, 2014 CFR

2014-07-01

... (CONTINUED) CHEMICAL ACCIDENT PREVENTION PROVISIONS Risk Management Plan § 68.165 Offsite consequence... released in pounds; (7) Release rate; (8) Release duration; (9) Wind speed and atmospheric stability class...

Coupled atmosphere-ocean-wave simulations of a storm event over the Gulf of Lion and Balearic Sea

USGS Publications Warehouse

Renault, Lionel; Chiggiato, Jacopo; Warner, John C.; Gomez, Marta; Vizoso, Guillermo; Tintore, Joaquin

2012-01-01

The coastal areas of the North-Western Mediterranean Sea are one of the most challenging places for ocean forecasting. This region is exposed to severe storms events that are of short duration. During these events, significant air-sea interactions, strong winds and large sea-state can have catastrophic consequences in the coastal areas. To investigate these air-sea interactions and the oceanic response to such events, we implemented the Coupled Ocean-Atmosphere-Wave-Sediment Transport Modeling System simulating a severe storm in the Mediterranean Sea that occurred in May 2010. During this event, wind speed reached up to 25 m.s-1 inducing significant sea surface cooling (up to 2°C) over the Gulf of Lion (GoL) and along the storm track, and generating surface waves with a significant height of 6 m. It is shown that the event, associated with a cyclogenesis between the Balearic Islands and the GoL, is relatively well reproduced by the coupled system. A surface heat budget analysis showed that ocean vertical mixing was a major contributor to the cooling tendency along the storm track and in the GoL where turbulent heat fluxes also played an important role. Sensitivity experiments on the ocean-atmosphere coupling suggested that the coupled system is sensitive to the momentum flux parameterization as well as air-sea and air-wave coupling. Comparisons with available atmospheric and oceanic observations showed that the use of the fully coupled system provides the most skillful simulation, illustrating the benefit of using a fully coupled ocean-atmosphere-wave model for the assessment of these storm events.

ENSO Bred Vectors in Coupled Ocean-Atmosphere General Circulation Models

NASA Technical Reports Server (NTRS)

Yang, S. C.; Cai, Ming; Kalnay, E.; Rienecker, M.; Yuan, G.; Toth, ZA.

2004-01-01

The breeding method has been implemented in the NASA Seasonal-to-Interannual Prediction Project (NSIPP) Coupled General Circulation Model (CGCM) with the goal of improving operational seasonal to interannual climate predictions through ensemble forecasting and data assimilation. The coupled instability as cap'tured by the breeding method is the first attempt to isolate the evolving ENSO instability and its corresponding global atmospheric response in a fully coupled ocean-atmosphere GCM. Our results show that the growth rate of the coupled bred vectors (BV) peaks at about 3 months before a background ENSO event. The dominant growing BV modes are reminiscent of the background ENSO anomalies and show a strong tropical response with wind/SST/thermocline interrelated in a manner similar to the background ENSO mode. They exhibit larger amplitudes in the eastern tropical Pacific, reflecting the natural dynamical sensitivity associated with the presence of the shallow thermocline. Moreover, the extratropical perturbations associated with these coupled BV modes reveal the variations related to the atmospheric teleconnection patterns associated with background ENSO variability, e.g. over the North Pacific and North America. A similar experiment was carried out with the NCEP/CFS03 CGCM. Comparisons between bred vectors from the NSIPP CGCM and NCEP/CFS03 CGCM demonstrate the robustness of the results. Our results strongly suggest that the breeding method can serve as a natural filter to identify the slowly varying, coupled instabilities in a coupled GCM, which can be used to construct ensemble perturbations for ensemble forecasts and to estimate the coupled background error covariance for coupled data assimilation.

An Investigation of Land-Atmosphere Coupling from Local to Regional Scales

NASA Astrophysics Data System (ADS)

Brunsell, N. A.; Van Vleck, E.; Rahn, D. A.

2017-12-01

The exchanges of mass and energy between the surface and atmosphere have been shown to depend upon both local and regional climatic influences. However, the degree of control exerted by the land surface on the coupling metrics is not well understood. In particular, we lack an understanding of the relationship between the local microclimate of a site and the regional forces responsible for land-atmosphere coupling. To address this, we investigate a series of metrics calculated from eddy covariance data and ceilometer data, land surface modeling and remotely sensed observations in the central United States to diagnose these interactions and predict the change from one coupling regime (e.g. wet/dry coupling) to another state. The stability of the coupling is quantified using a Lyapunov exponent based methodology. Through the use of a wavelet information theoretic approach, we isolate the roles local energy partitioning, as well as the temperature and moisture gradients on controlling and changing the coupling regime. Taking a multi-scale observational approach, we first examine the relationship at the tower scale. Using land surface models, we quantify to what extent current models are capable of properly diagnosing the dynamics of the coupling regime. In particular, we focus on the role of the surface moisture and vegetation to initiate and maintain precipitation feedbacks. We extend this analysis to the regional scale by utilizing reanalysis and remotely sensed observations. Thus, we are able to quantify the changes in observed coupling patterns with linkages to local interactions to address the question of the local control that the surface exerts over the maintenance of land-atmosphere coupling.

The vector radiative transfer numerical model of coupled ocean-atmosphere system using the matrix-operator method

NASA Astrophysics Data System (ADS)

Xianqiang, He; Delu, Pan; Yan, Bai; Qiankun, Zhu

2005-10-01

The numerical model of the vector radiative transfer of the coupled ocean-atmosphere system is developed based on the matrix-operator method, which is named PCOART. In PCOART, using the Fourier analysis, the vector radiative transfer equation (VRTE) splits up into a set of independent equations with zenith angle as only angular coordinate. Using the Gaussian-Quadrature method, VRTE is finally transferred into the matrix equation, which is calculated by using the adding-doubling method. According to the reflective and refractive properties of the ocean-atmosphere interface, the vector radiative transfer numerical model of ocean and atmosphere is coupled in PCOART. By comparing with the exact Rayleigh scattering look-up-table of MODIS(Moderate-resolution Imaging Spectroradiometer), it is shown that PCOART is an exact numerical calculation model, and the processing methods of the multi-scattering and polarization are correct in PCOART. Also, by validating with the standard problems of the radiative transfer in water, it is shown that PCOART could be used to calculate the underwater radiative transfer problems. Therefore, PCOART is a useful tool to exactly calculate the vector radiative transfer of the coupled ocean-atmosphere system, which can be used to study the polarization properties of the radiance in the whole ocean-atmosphere system and the remote sensing of the atmosphere and ocean.

What's new in the Atmospheric Model Evaluation Tool (AMET) version 1.3

EPA Science Inventory

A new version of the Atmospheric Model Evaluation Tool (AMET) has been released. The new version of AMET, version 1.3 (AMETv1.3), contains a number of updates and changes from the previous of version of AMET (v1.2) released in 2012. First, the Perl scripts used in the previous ve...

Lithosphere-Atmosphere coupling: Spectral element modeling of the evolution of acoustic waves in the atmosphere from an underground source.

NASA Astrophysics Data System (ADS)

Averbuch, Gil; Price, Colin

2015-04-01

Lithosphere-Atmosphere coupling: Spectral element modeling of the evolution of acoustic waves in the atmosphere from an underground source. G. Averbuch, C. Price Department of Geosciences, Tel Aviv University, Israel Infrasound is one of the four Comprehensive Nuclear-Test Ban Treaty technologies for monitoring nuclear explosions. This technology measures the acoustic waves generated by the explosions followed by their propagation through the atmosphere. There are also natural phenomena that can act as an infrasound sources like sprites, volcanic eruptions and earthquakes. The infrasound waves generated from theses phenomena can also be detected by the infrasound arrays. In order to study the behavior of these waves, i.e. the physics of wave propagation in the atmosphere, their evolution and their trajectories, numerical methods are required. This presentation will deal with the evolution of acoustic waves generated by underground sources (earthquakes and underground explosions). A 2D Spectral elements formulation for lithosphere-atmosphere coupling will be presented. The formulation includes the elastic wave equation for the seismic waves and the momentum, mass and state equations for the acoustic waves in a moving stratified atmosphere. The coupling of the two media is made by boundary conditions that ensures the continuity of traction and velocity (displacement) in the normal component to the interface. This work has several objectives. The first is to study the evolution of acoustic waves in the atmosphere from an underground source. The second is to derive transmission coefficients for the energy flux with respect to the seismic magnitude and earth density. The third will be the generation of seismic waves from acoustic waves in the atmosphere. Is it possible?

Studies of regional-scale climate variability and change. Hidden Markov models and coupled ocean-atmosphere modes

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ghil, M.; Kravtsov, S.; Robertson, A. W.

2008-10-14

This project was a continuation of previous work under DOE CCPP funding, in which we had developed a twin approach of probabilistic network (PN) models (sometimes called dynamic Bayesian networks) and intermediate-complexity coupled ocean-atmosphere models (ICMs) to identify the predictable modes of climate variability and to investigate their impacts on the regional scale. We had developed a family of PNs (similar to Hidden Markov Models) to simulate historical records of daily rainfall, and used them to downscale GCM seasonal predictions. Using an idealized atmospheric model, we had established a novel mechanism through which ocean-induced sea-surface temperature (SST) anomalies might influencemore » large-scale atmospheric circulation patterns on interannual and longer time scales; we had found similar patterns in a hybrid coupled ocean-atmosphere-sea-ice model. The goal of the this continuation project was to build on these ICM results and PN model development to address prediction of rainfall and temperature statistics at the local scale, associated with global climate variability and change, and to investigate the impact of the latter on coupled ocean-atmosphere modes. Our main results from the grant consist of extensive further development of the hidden Markov models for rainfall simulation and downscaling together with the development of associated software; new intermediate coupled models; a new methodology of inverse modeling for linking ICMs with observations and GCM results; and, observational studies of decadal and multi-decadal natural climate results, informed by ICM results.« less

Coupled Regional Ocean-Atmosphere Modeling of the Mount Pinatubo Impact on the Red Sea

NASA Astrophysics Data System (ADS)

Stenchikov, G. L.; Osipov, S.

2017-12-01

The 1991 eruption of Mount Pinatubo had dramatic effects on the regional climate in the Middle East. Though acknowledged, these effects have not been thoroughly studied. To fill this gap and to advance understanding of the mechanisms that control variability in the Middle East's regional climate, we simulated the impact of the 1991 Pinatubo eruption using a regional coupled ocean-atmosphere modeling system set for the Middle East and North Africa (MENA) domain. We used the Coupled Ocean-Atmosphere-Wave-Sediment Transport (COAWST) framework, which couples the Weather Research and Forecasting Model (WRF) model with the Regional Oceanic Modeling System (ROMS). We modified the WRF model to account for the radiative effect of volcanic aerosols. Our coupled ocean-atmosphere simulations verified by available observations revealed strong perturbations in the energy balance of the Red Sea, which drove thermal and circulation responses. Our modeling approach allowed us to separate changes in the atmospheric circulation caused by the impact of the volcano from direct regional radiative cooling from volcanic aerosols. The atmospheric circulation effect was significantly stronger than the direct volcanic aerosols effect. We found that the Red Sea response to the Pinatubo eruption was stronger and qualitatively different from that of the global ocean system. Our results suggest that major volcanic eruptions significantly affect the climate in the Middle East and the Red Sea and should be carefully taken into account in assessments of long-term climate variability and warming trends in MENA and the Red Sea.

Is the extent of glaciation limited by marine gas-hydrates?

USGS Publications Warehouse

Paull, Charles K.; Ussler, William; Dillon, William P.

1991-01-01

Methane may have been released to the atmosphere during the Quaternary from Arctic shelf gas-hydrates as a result of thermal decomposition caused by climatic warming and rising sea-level; this release of methane (a greenhouse gas) may represent a positive feedback on global warming [Revelle, 1983; Kvenvolden, 1988a; Nisbet, 1990]. We consider the response to sea-level changes by the immense amount of gas-hydrate that exists in continental rise sediments, and suggest that the reverse situation may apply—that release of methane trapped in the deep-sea sediments as gas-hydrates may provide a negative feedback to advancing glaciation. Methane is likely to be released from deep-sea gas-hydrates as sea-level falls because methane gas-hydrates decompose with pressure decrease. Methane would be released to sediment pore space at shallow sub-bottom depths (100's of meters beneath the seafloor, commonly at water depths of 500 to 4,000 m) producing zones of markedly decreased sediment strength, leading to slumping [Carpenter, 1981; Kayen, 1988] and abrupt release of the gas. Methane is likely to be released to the atmosphere in spikes that become larger and more frequent as glaciation progresses. Because addition of methane to the atmosphere warms the planet, this process provides a negative feedback to glaciation, and could trigger deglaciation.

Climate sensitivity derived from orbital-scale, δ11B-based pCO2 estimates in the early Pleistocene, ~1.5 Ma

NASA Astrophysics Data System (ADS)

Dyez, K. A.; Hoenisch, B.

2015-12-01

Atmospheric CO2 concentrations in the late Pleistocene have been characterized from ancient air bubbles trapped within polar ice sheets. Ice-core records clearly demonstrate the glacial-interglacial relationship between the global carbon cycle and climate, but they are so far limited to the last 800 ky, when glacial cycles occurred approximately every 100-ky. Boron isotope ratios (δ11B) recorded in the tests of fossil planktic foraminifera offer an opportunity to extend the atmospheric pCO2 record into the early Pleistocene, when glacial cycles instead occurred approximately every 41-ky. We present a new high-resolution record of planktic foraminiferal d11B, Mg/Ca (a sea surface temperature proxy) and salinity estimates from the deconvolution of δ18O and Mg/Ca. Combined with reasonable assumptions of ocean alkalinity, these data allow us to estimate pCO2 over three of the 41-ky climate cycles at ~1.5 Ma. Our results confirm the hypothesis that climate and atmospheric pCO2 were coupled beyond ice core records and provide new constraints for studies of long-term CO2 storage and release, regional controls on the early Pleistocene carbon cycle, and estimating climate sensitivity before the mid-Pleistocene transition.

A COMPREHENSIVE ANALYSIS OF CHLORINE TRANSPORT AND FATE FOLLOWING A LARGE ENVIRONMENTAL RELEASE

DOE Office of Scientific and Technical Information (OSTI.GOV)

Buckley, R.; Hunter, C.; Werth, D.

2011-05-10

A train derailment occurred in Graniteville, South Carolina during the early morning of January 6, 2005, and resulted in the release of a large amount of cryogenic pressurized liquid chlorine to the environment in a short time period. A comprehensive evaluation of the transport and fate of the released chlorine was performed, accounting for dilution, diffusion, transport and deposition into the local environment. This involved the characterization of a three-phased chlorine release, a detailed determination of local atmospheric mechanisms acting on the released chlorine, the establishment of atmospheric-hydrological physical exchange mechanisms, and aquatic dilution and mixing. This presentation will providemore » an overview of the models used in determining the total air-to-water mass transfer estimated to have occurred as a result of the roughly 60 tons of chlorine released into the atmosphere from the train derailment. The assumptions used in the modeling effort will be addressed, along with a comparison with available observational data to validate the model results. Overall, model-estimated chlorine concentrations in the airborne plume compare well with human and animal exposure data collected in the days after the derailment.« less

Atmospheric Dispersion Modeling of the February 2014 Waste Isolation Pilot Plant Release

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nasstrom, John; Piggott, Tom; Simpson, Matthew

2015-07-22

This report presents the results of a simulation of the atmospheric dispersion and deposition of radioactivity released from the Waste Isolation Pilot Plant (WIPP) site in New Mexico in February 2014. These simulations were made by the National Atmospheric Release Advisory Center (NARAC) at Lawrence Livermore National Laboratory (LLNL), and supersede NARAC simulation results published in a previous WIPP report (WIPP, 2014). The results presented in this report use additional, more detailed data from WIPP on the specific radionuclides released, radioactivity release amounts and release times. Compared to the previous NARAC simulations, the new simulation results in this report aremore » based on more detailed modeling of the winds, turbulence, and particle dry deposition. In addition, the initial plume rise from the exhaust vent was considered in the new simulations, but not in the previous NARAC simulations. The new model results show some small differences compared to previous results, but do not change the conclusions in the WIPP (2014) report. Presented are the data and assumptions used in these model simulations, as well as the model-predicted dose and deposition on and near the WIPP site. A comparison of predicted and measured radionuclide-specific air concentrations is also presented.« less

Radiocesium in the Savannah River Site environment.

PubMed

Carlton, W H; Murphy, C E; Evans, A G

1994-09-01

The Savannah River Site has produced plutonium, tritium, and other special nuclear materials for national defense, other government programs, and some civilian purposes. Radiocesium, a waste product, has been released to the environment during the operation of five reactors, two radio-chemical processing facilities, and a high-level waste storage system. During the period 1955-1989, 130 GBq of 137Cs was released to the atmosphere and 2.2 x 10(4) GBq was released to site streams and ponds. Approximately 65% of the latter remained on the site. The maximum individual effective dose equivalent at the site boundary was estimated to be 3.3 microSv from atmospheric releases and 600 microSv from liquid releases. The 80-km population dose was 1.6 person-Sv.

The Impact of Air-Sea Interactions on the Representation of Tropical Precipitation Extremes

NASA Astrophysics Data System (ADS)

Hirons, L. C.; Klingaman, N. P.; Woolnough, S. J.

2018-02-01

The impacts of air-sea interactions on the representation of tropical precipitation extremes are investigated using an atmosphere-ocean-mixed-layer coupled model. The coupled model is compared to two atmosphere-only simulations driven by the coupled-model sea-surface temperatures (SSTs): one with 31 day running means (31 d), the other with a repeating mean annual cycle. This allows separation of the effects of interannual SST variability from those of coupled feedbacks on shorter timescales. Crucially, all simulations have a consistent mean state with very small SST biases against present-day climatology. 31d overestimates the frequency, intensity, and persistence of extreme tropical precipitation relative to the coupled model, likely due to excessive SST-forced precipitation variability. This implies that atmosphere-only attribution and time-slice experiments may overestimate the strength and duration of precipitation extremes. In the coupled model, air-sea feedbacks damp extreme precipitation, through negative local thermodynamic feedbacks between convection, surface fluxes, and SST.

Effect of land model ensemble versus coupled model ensemble on the simulation of precipitation climatology and variability

NASA Astrophysics Data System (ADS)

Wei, Jiangfeng; Dirmeyer, Paul A.; Yang, Zong-Liang; Chen, Haishan

2017-10-01

Through a series of model simulations with an atmospheric general circulation model coupled to three different land surface models, this study investigates the impacts of land model ensembles and coupled model ensemble on precipitation simulation. It is found that coupling an ensemble of land models to an atmospheric model has a very minor impact on the improvement of precipitation climatology and variability, but a simple ensemble average of the precipitation from three individually coupled land-atmosphere models produces better results, especially for precipitation variability. The generally weak impact of land processes on precipitation should be the main reason that the land model ensembles do not improve precipitation simulation. However, if there are big biases in the land surface model or land surface data set, correcting them could improve the simulated climate, especially for well-constrained regional climate simulations.

GLACE: The Global Land-Atmosphere Coupling Experiment Part 2: Analysis

NASA Technical Reports Server (NTRS)

Guo, Zhichang; Dirmeyer, Paul A.; Koster, Randal D.; Bonan, Gordon; Chan, Edmond; Cox, Peter; Gordon, C. T.; Kanae, Shinjiro; Kowalczyk, Eva; Lawrence, David

2005-01-01

The twelve weather and climate models participating in the Global Land-Atmosphere Coupling Experiment (GLACE) show both a wide variation in the strength of land-atmosphere coupling and some intriguing commonalities. In this paper, we address the causes of variations in coupling strength - both the geographic variations within a given model and the model-to-model differences. The ability of soil moisture to affect precipitation is examined in two stages, namely, the ability of the soil moisture to affect evaporation, and the ability of evaporation to affect precipitation. Most of the differences between the models and within a given model are found to be associated with the first stage - an evaporation rate that varies strongly and consistently with soil moisture tends to lead to a higher coupling strength. The first stage differences reflect identifiable differences in model parameterization and model climate. Intermodel differences in the evaporation-precipitation connection, however, also play a key role.

Interannual rainfall variability over China in the MetUM GA6 and GC2 configurations

NASA Astrophysics Data System (ADS)

Stephan, Claudia Christine; Klingaman, Nicholas P.; Vidale, Pier Luigi; Turner, Andrew G.; Demory, Marie-Estelle; Guo, Liang

2018-05-01

Six climate simulations of the Met Office Unified Model Global Atmosphere 6.0 and Global Coupled 2.0 configurations are evaluated against observations and reanalysis data for their ability to simulate the mean state and year-to-year variability of precipitation over China. To analyse the sensitivity to air-sea coupling and horizontal resolution, atmosphere-only and coupled integrations at atmospheric horizontal resolutions of N96, N216 and N512 (corresponding to ˜ 200, 90 and 40 km in the zonal direction at the equator, respectively) are analysed. The mean and interannual variance of seasonal precipitation are too high in all simulations over China but improve with finer resolution and coupling. Empirical orthogonal teleconnection (EOT) analysis is applied to simulated and observed precipitation to identify spatial patterns of temporally coherent interannual variability in seasonal precipitation. To connect these patterns to large-scale atmospheric and coupled air-sea processes, atmospheric and oceanic fields are regressed onto the corresponding seasonal mean time series. All simulations reproduce the observed leading pattern of interannual rainfall variability in winter, spring and autumn; the leading pattern in summer is present in all but one simulation. However, only in two simulations are the four leading patterns associated with the observed physical mechanisms. Coupled simulations capture more observed patterns of variability and associate more of them with the correct physical mechanism, compared to atmosphere-only simulations at the same resolution. However, finer resolution does not improve the fidelity of these patterns or their associated mechanisms. This shows that evaluating climate models by only geographical distribution of mean precipitation and its interannual variance is insufficient. The EOT analysis adds knowledge about coherent variability and associated mechanisms.

Online coupled regional meteorology-chemistry models in Europe: current status and prospects

NASA Astrophysics Data System (ADS)

Baklanov, A.; Schluenzen, K. H.; Suppan, P.; Baldasano, J.; Brunner, D.; Aksoyoglu, S.; Carmichael, G.; Douros, J.; Flemming, J.; Forkel, R.; Galmarini, S.; Gauss, M.; Grell, G.; Hirtl, M.; Joffre, S.; Jorba, O.; Kaas, E.; Kaasik, M.; Kallos, G.; Kong, X.; Korsholm, U.; Kurganskiy, A.; Kushta, J.; Lohmann, U.; Mahura, A.; Manders-Groot, A.; Maurizi, A.; Moussiopoulos, N.; Rao, S. T.; Savage, N.; Seigneur, C.; Sokhi, R.; Solazzo, E.; Solomos, S.; Sørensen, B.; Tsegas, G.; Vignati, E.; Vogel, B.; Zhang, Y.

2013-05-01

The simulation of the coupled evolution of atmospheric dynamics, pollutant transport, chemical reactions and atmospheric composition is one of the most challenging tasks in environmental modelling, climate change studies, and weather forecasting for the next decades as they all involve strongly integrated processes. Weather strongly influences air quality (AQ) and atmospheric transport of hazardous materials, while atmospheric composition can influence both weather and climate by directly modifying the atmospheric radiation budget or indirectly affecting cloud formation. Until recently, however, due to the scientific complexities and lack of computational power, atmospheric chemistry and weather forecasting have developed as separate disciplines, leading to the development of separate modelling systems that are only loosely coupled. The continuous increase in computer power has now reached a stage that enables us to perform online coupling of regional meteorological models with atmospheric chemical transport models. The focus on integrated systems is timely, since recent research has shown that meteorology and chemistry feedbacks are important in the context of many research areas and applications, including numerical weather prediction (NWP), AQ forecasting as well as climate and Earth system modelling. However, the relative importance of online integration and its priorities, requirements and levels of detail necessary for representing different processes and feedbacks can greatly vary for these related communities: (i) NWP, (ii) AQ forecasting and assessments, (iii) climate and earth system modelling. Additional applications are likely to benefit from online modelling, e.g.: simulation of volcanic ash or forest fire plumes, pollen warnings, dust storms, oil/gas fires, geo-engineering tests involving changes in the radiation balance. The COST Action ES1004 - European framework for online integrated air quality and meteorology modelling (EuMetChem) - aims at paving the way towards a new generation of online integrated atmospheric chemical transport and meteorology modelling with two-way interactions between different atmospheric processes including dynamics, chemistry, clouds, radiation, boundary layer and emissions. As its first task, we summarise the current status of European modelling practices and experience with online coupled modelling of meteorology with atmospheric chemistry including feedback mechanisms and attempt reviewing the various issues connected to the different modules of such online coupled models but also providing recommendations for coping with them for the benefit of the modelling community at large.

Chemistry of Earth's Putative Steam Atmosphere

NASA Astrophysics Data System (ADS)

Fegley, B.; Schaefer, L.

2007-12-01

The concept of a steam atmosphere generated by impact devolatilization of planetesimals accreted during Earth's formation is over 20 years old (Matsui and Abe, 1986; Lange and Ahrens, 1982). Surprisingly, with the possible exception of a few qualitative remarks, no one has critically assessed this scenario. We use thermochemical equilibrium and, where relevant, thermochemical kinetic calculations to model the chemistry of the "steam" atmosphere produced by impact volatilization of different types of accreting material. We present results for our nominal conditions (1500 K, total P = 100 bar). We also studied the effects of variable temperature and total pressure. The composition of the accreting material is modeled using average compositions of the Orgueil CI chondrite, the Murchison CM2 chondrite, the Allende CV3 chondrite, average ordinary (H, L, LL) chondrites, and average enstatite (EH, EL) chondrites. The major gases released from CI and CM chondritic material are H2O, CO2, H2, H2S, CO, CH4, and SO2 in decreasing order of abundance. About 10% of the atmosphere is CO2. The major gases released from CV chondritic material are CO2, H2O, CO, H2, and SO2 in decreasing order of abundance. About 20% of the total atmosphere is steam. The major gases released from average ordinary chondritic material are H2, CO, H2O, CO2, CH4, H2S, and N2 in decreasing order of abundance. The "steam" atmosphere is predominantly H2 + CO with steam being about 10% of the total atmosphere. The major gases released from EH chondritic material are H2, CO, H2O, CO2, N2, and CH4 in decreasing order of abundance. The "steam" atmosphere is predominantly H2 + CO with about 10% of the total atmosphere as steam. This work was supported by the NASA Astrobiology and Origins Programs.

The Sample Analysis at Mars Investigation and Instrument Suite

NASA Technical Reports Server (NTRS)

Mahaffy, Paul; Webster, Christopher R.; Conrad, Pamela G.; Arvey, Robert; Bleacher, Lora; Brinckerhoff, William B.; Eigenbrode, Jennifer L.; Chalmers, Robert A.; Dworkin, Jason P.; Errigo, Therese;

Thermosphere Dynamics Workshop, volume 2

NASA Technical Reports Server (NTRS)

Mayr, H. G. (Editor); Miller, N. J. (Editor)

1986-01-01

Atmospheric observations reported on include recent measurements of thermospherical composition, gas temperatures, auroral emissions, ion-neutral collisional coupling, electric fields, and plasma convection. Theoretical studies reported on include model calculations of thermospherical general circulation, thermospheric tides, thermospheric tidal coupling to the lower atmosphere, interactions between thermospheic chemistry and dynamics and thermosphere-ionosphere coupling processes. The abstracts provide details given in each talk but the figures represent the fundamental information exchanged within the workshop

Atmospheric chemistry of hydrogen fluoride

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cheng, Meng -Dawn

In this study, the atmospheric chemistry, emissions, and surface boundary layer transport of hydrogen fluoride (HF) is summarized. Although HF is known to be chemically reactive and highly soluble, both factors affect transport and removal in the atmosphere, we suggest that the chemistry can be ignored when the HF concentration is at a sufficiently low level (e.g., 10 ppmv). At a low concentration, the capability for HF to react in the atmosphere is diminished and therefore the species can be mathematically treated as inert during the transport. At a sufficiently high concentration of HF (e.g., kg/s release rate and thousandsmore » of ppm), however, HF can go through a series of rigorous chemical reactions including polymerization, depolymerization, and reaction with water to form molecular complex. As such, the HF species cannot be considered as inert because the reactions could intimately influence the plume s thermodynamic properties affecting the changes in plume temperature and density. The atmospheric residence time of HF was found to be less than four (4) days, and deposition (i.e., atmosphere to surface transport) is the dominant mechanism that controls the removal of HF and its oligomers from the atmosphere. The literature data on HF dry deposition velocity was relatively high compared to many commonly found atmospheric species such as ozone, sulfur dioxide, nitrogen oxides, etc. The global average of wet deposition velocity of HF was found to be zero based on one literature source. Uptake of HF by rain drops is limited by the acidity of the rain drops, and atmospheric particulate matter contributes negligibly to HF uptake. Finally, given that the reactivity of HF at a high release rate and elevated mole concentration cannot be ignored, it is important to incorporate the reaction chemistry in the near-field dispersion close to the proximity of the release source, and to incorporate the deposition mechanism in the far-field dispersion away from the release source. In other words, a hybrid computational scheme may be needed to address transport and atmospheric chemistry of HF in a range of applications. The model uncertainty will be limited by the precision of boundary layer parameterization and ability to accurately model the atmospheric turbulence.« less

Atmospheric chemistry of hydrogen fluoride

DOE PAGES

Cheng, Meng -Dawn

2017-04-11

In this study, the atmospheric chemistry, emissions, and surface boundary layer transport of hydrogen fluoride (HF) is summarized. Although HF is known to be chemically reactive and highly soluble, both factors affect transport and removal in the atmosphere, we suggest that the chemistry can be ignored when the HF concentration is at a sufficiently low level (e.g., 10 ppmv). At a low concentration, the capability for HF to react in the atmosphere is diminished and therefore the species can be mathematically treated as inert during the transport. At a sufficiently high concentration of HF (e.g., kg/s release rate and thousandsmore » of ppm), however, HF can go through a series of rigorous chemical reactions including polymerization, depolymerization, and reaction with water to form molecular complex. As such, the HF species cannot be considered as inert because the reactions could intimately influence the plume s thermodynamic properties affecting the changes in plume temperature and density. The atmospheric residence time of HF was found to be less than four (4) days, and deposition (i.e., atmosphere to surface transport) is the dominant mechanism that controls the removal of HF and its oligomers from the atmosphere. The literature data on HF dry deposition velocity was relatively high compared to many commonly found atmospheric species such as ozone, sulfur dioxide, nitrogen oxides, etc. The global average of wet deposition velocity of HF was found to be zero based on one literature source. Uptake of HF by rain drops is limited by the acidity of the rain drops, and atmospheric particulate matter contributes negligibly to HF uptake. Finally, given that the reactivity of HF at a high release rate and elevated mole concentration cannot be ignored, it is important to incorporate the reaction chemistry in the near-field dispersion close to the proximity of the release source, and to incorporate the deposition mechanism in the far-field dispersion away from the release source. In other words, a hybrid computational scheme may be needed to address transport and atmospheric chemistry of HF in a range of applications. The model uncertainty will be limited by the precision of boundary layer parameterization and ability to accurately model the atmospheric turbulence.« less

A sensitivity study of the coupled simulation of the Northeast Brazil rainfall variability

NASA Astrophysics Data System (ADS)

Misra, Vasubandhu

2007-06-01

Two long-term coupled ocean-land-atmosphere simulations with slightly different parameterization of the diagnostic shallow inversion clouds in the atmospheric general circulation model (AGCM) of the Center for Ocean-Land-Atmosphere Studies (COLA) coupled climate model are compared for their annual cycle and interannual variability of the northeast Brazil (NEB) rainfall variability. It is seen that the solar insolation affected by the changes to the shallow inversion clouds results in large scale changes to the gradients of the SST and the surface pressure. The latter in turn modulates the surface convergence and the associated Atlantic ITCZ precipitation and the NEB annual rainfall variability. In contrast, the differences in the NEB interannual rainfall variability between the two coupled simulations is attributed to their different remote ENSO forcing.

CO2 co-gasification of lower sulphur petroleum coke and sugar cane bagasse via TG-FTIR analysis technique.

PubMed

Edreis, Elbager M A; Luo, Guangqian; Li, Aijun; Chao, Chen; Hu, Hongyun; Zhang, Sen; Gui, Ben; Xiao, Li; Xu, Kai; Zhang, Pingan; Yao, Hong

2013-05-01

This study investigates the non-isothermal mechanism and kinetic behaviour of gasification of a lower sulphur petroleum coke, sugar cane bagasse and blends under carbon dioxide atmosphere conditions using the thermogravimetric analyser (TGA). The gas products were measured online with coupled Fourier transform infrared spectroscopy (FTIR). The achieved results explored that the sugar cane bagasse and blend gasification happened in two steps: at (<500 °C) the volatiles are released, and at (>700 °C) char gasification occurred, whereas the lower sulphur petroleum coke presented only one char gasification stage at (>800 °C). Significant interactions were observed in the whole process. Some solid-state mechanisms were studied by the Coats-Redfern method in order to observe the mechanisms responsible for the gasification of samples. The results show that the chemical first order reaction is the best responsible mechanism for whole process. The main released gases are CO2, CO, CH4, HCOOH, C6H5OH and CH3COOH. Copyright © 2013 Elsevier Ltd. All rights reserved.

Infrasound induced instability by modulation of condensation process in the atmosphere.

PubMed

Naugolnykh, Konstantin; Rybak, Samuil

2008-12-01

A sound wave in supersaturated water vapor can modulate both the process of heat release caused by condensation, and subsequently, as a result, the resonance interaction of sound with the modulated heat release provides sound amplification. High-intensity atmospheric perturbations such as cyclones and thunderstorms generate infrasound, which is detectable at large distances from the source. The wave-condensation instability can lead to variation in the level of infrasound radiation by a developing cyclone, and this can be as a precursor of these intense atmospheric events.

Automated life-detection experiments for the Viking mission to Mars

NASA Technical Reports Server (NTRS)

Klein, H. P.

1974-01-01

As part of the Viking mission to Mars in 1975, an automated set of instruments is being built to test for the presence of metabolizing organisms on that planet. Three separate modules are combined in this instrument so that samples of the Martian surface can be subjected to a broad array of experimental conditions so as to measure biological activity. The first, the Pyrolytic Release Module, will expose surface samples to a mixture of C-14O and C-14O2 in the presence of Martian atmosphere and a light source that simulates the Martian visible spectrum. The assay system is designed to determine the extent of assimilation of CO or CO2 into organic compounds. The Gas Exchange Module will incubate surface samples in a humidified CO2 atmosphere. At specified times, portions of the incubation atmosphere will be analyzed by gas chromatography to detect the release or uptake of CO2 and several additional gases. The Label Release Module will incubate surface samples with a dilute aqueous solution of simple radioactive organic substrates in Martian atmosphere, and the gas phase will be monitored continuously for the release of labeled CO2.

Natural chlorine and fluorine in the atmosphere, water and precipitation

NASA Technical Reports Server (NTRS)

Friend, James P.

1990-01-01

The geochemical cycles of chlorine and fluorine are surveyed and summarized as framework for the understanding of the global natural abundances of these species in the atmosphere, water, and precipitation. In the cycles the fluxes into and out of the atmosphere can be balanced within the limits of our knowledge of the natural sources and sinks. Sea salt from the ocean surfaces represent the predominant portion of the source of chlorine. It is also an important source of atmospheric fluorine, but volcanoes are likely to be more important fluorine sources. Dry deposition of sea salt returns about 85 percent of the salt released there. Precipitation removes the remainder. Most of the sea salt materials are considered to be cyclic, moving through sea spray over the oceans and either directly back to the oceans or deposited dry and in precipitation on land, whence it runs off into rivers and streams and returns to the oceans. Most of the natural chlorine in the atmosphere is in the form of particulate chloride ion with lesser amounts as gaseous inorganic chloride and methyl chloride vapor. Fluorine is emitted from volcanoes primarily as HF. It is possible that HF may be released directly form the ocean surface but this has not been confirmed by observation. HCl and most likely HF gases are released into the atmosphere by sea salt aerosols. The mechanism for the release is likely to be the provision of protons from the so-called excess sulfate and HNO3. Sea salt aerosol contains fluorine as F(-), MgF(+), CaF(+), and NaF. The concentrations of the various species of chlorine and fluorine that characterize primarily natural, unpolluted atmospheres are summarized in tables and are discussed in relation to their fluxes through the geochemical cycle.

PTR-ToF-MS Coupled with an Automated Sampling System and Tailored Data Analysis for Food Studies: Bioprocess Monitoring, Screening and Nose-space Analysis.

PubMed

Capozzi, Vittorio; Yener, Sine; Khomenko, Iuliia; Farneti, Brian; Cappellin, Luca; Gasperi, Flavia; Scampicchio, Matteo; Biasioli, Franco

2017-05-11

Proton Transfer Reaction (PTR), combined with a Time-of-Flight (ToF) Mass Spectrometer (MS) is an analytical approach based on chemical ionization that belongs to the Direct-Injection Mass Spectrometric (DIMS) technologies. These techniques allow the rapid determination of volatile organic compounds (VOCs), assuring high sensitivity and accuracy. In general, PTR-MS requires neither sample preparation nor sample destruction, allowing real time and non-invasive analysis of samples. PTR-MS are exploited in many fields, from environmental and atmospheric chemistry to medical and biological sciences. More recently, we developed a methodology based on coupling PTR-ToF-MS with an automated sampler and tailored data analysis tools, to increase the degree of automation and, consequently, to enhance the potential of the technique. This approach allowed us to monitor bioprocesses (e.g. enzymatic oxidation, alcoholic fermentation), to screen large sample sets (e.g. different origins, entire germoplasms) and to analyze several experimental modes (e.g. different concentrations of a given ingredient, different intensities of a specific technological parameter) in terms of VOC content. Here, we report the experimental protocols exemplifying different possible applications of our methodology: i.e. the detection of VOCs released during lactic acid fermentation of yogurt (on-line bioprocess monitoring), the monitoring of VOCs associated with different apple cultivars (large-scale screening), and the in vivo study of retronasal VOC release during coffee drinking (nosespace analysis).

The role of soil moisture in land surface-atmosphere coupling: climate model sensitivity experiments over India

NASA Astrophysics Data System (ADS)

Williams, Charles; Turner, Andrew

2015-04-01

It is generally acknowledged that anthropogenic land use changes, such as a shift from forested land into irrigated agriculture, may have an impact on regional climate and, in particular, rainfall patterns in both time and space. India provides an excellent example of a country in which widespread land use change has occurred during the last century, as the country tries to meet its growing demand for food. Of primary concern for agriculture is the Indian summer monsoon (ISM), which displays considerable seasonal and subseasonal variability. Although it is evident that changing rainfall variability will have a direct impact on land surface processes (such as soil moisture variability), the reverse impact is less well understood. However, the role of soil moisture in the coupling between the land surface and atmosphere needs to be properly explored before any potential impact of changing soil moisture variability on ISM rainfall can be understood. This paper attempts to address this issue, by conducting a number of sensitivity experiments using a state-of-the-art climate model from the UK Meteorological Office Hadley Centre: HadGEM2. Several experiments are undertaken, with the only difference between them being the extent to which soil moisture is coupled to the atmosphere. Firstly, the land surface is fully coupled to the atmosphere, globally (as in standard model configurations); secondly, the land surface is entirely uncoupled from the atmosphere, again globally, with soil moisture values being prescribed on a daily basis; thirdly, the land surface is uncoupled from the atmosphere over India but fully coupled elsewhere; and lastly, vice versa (i.e. the land surface is coupled to the atmosphere over India but uncoupled elsewhere). Early results from this study suggest certain 'hotspot' regions where the impact of soil moisture coupling/uncoupling may be important, and many of these regions coincide with previous studies. Focusing on the third experiment, i.e. uncoupled over India and coupled elsewhere, preliminary results suggest an increase in rainfall, surface temperature and pressure over northern India and the Himalayas, as well as a decrease in rainfall over the Bay of Bengal and the Maritime Continent. Other metrics, such as the northward propagation of intraseasonal rainfall variability and sensible and latent heat fluxes, are also discussed.

Effects of air-sea interaction on extended-range prediction of geopotential height at 500 hPa over the northern extratropical region

NASA Astrophysics Data System (ADS)

Wang, Xujia; Zheng, Zhihai; Feng, Guolin

2018-04-01

The contribution of air-sea interaction on the extended-range prediction of geopotential height at 500 hPa in the northern extratropical region has been analyzed with a coupled model form Beijing Climate Center and its atmospheric components. Under the assumption of the perfect model, the extended-range prediction skill was evaluated by anomaly correlation coefficient (ACC), root mean square error (RMSE), and signal-to-noise ratio (SNR). The coupled model has a better prediction skill than its atmospheric model, especially, the air-sea interaction in July made a greater contribution for the improvement of prediction skill than other months. The prediction skill of the extratropical region in the coupled model reaches 16-18 days in all months, while the atmospheric model reaches 10-11 days in January, April, and July and only 7-8 days in October, indicating that the air-sea interaction can extend the prediction skill of the atmospheric model by about 1 week. The errors of both the coupled model and the atmospheric model reach saturation in about 20 days, suggesting that the predictable range is less than 3 weeks.

Omens of coupled model biases in the CMIP5 AMIP simulations

NASA Astrophysics Data System (ADS)

Găinuşă-Bogdan, Alina; Hourdin, Frédéric; Traore, Abdoul Khadre; Braconnot, Pascale

2018-02-01

Despite decades of efforts and improvements in the representation of processes as well as in model resolution, current global climate models still suffer from a set of important, systematic biases in sea surface temperature (SST), not much different from the previous generation of climate models. Many studies have looked at errors in the wind field, cloud representation or oceanic upwelling in coupled models to explain the SST errors. In this paper we highlight the relationship between latent heat flux (LH) biases in forced atmospheric simulations and the SST biases models develop in coupled mode, at the scale of the entire intertropical domain. By analyzing 22 pairs of forced atmospheric and coupled ocean-atmosphere simulations from the CMIP5 database, we show a systematic, negative correlation between the spatial patterns of these two biases. This link between forced and coupled bias patterns is also confirmed by two sets of dedicated sensitivity experiments with the IPSL-CM5A-LR model. The analysis of the sources of the atmospheric LH bias pattern reveals that the near-surface wind speed bias dominates the zonal structure of the LH bias and that the near-surface relative humidity dominates the east-west contrasts.

Observed Local Soil Moisture-Atmosphere Feedbacks within the Context of Remote SST Anomalies: Lessons From Recent Droughts

NASA Astrophysics Data System (ADS)

Tawfik, A. B.; Dirmeyer, P.; Lawrence, D. M.

2015-12-01

The existence and possible transition from positive to negative soil moisture-atmosphere feedbacks is explored in this presentation using collocated flux tower measurements (Ameriflux) and atmospheric profiles from reanalysis. The focus is on the series of physical processes that lead to these local feedbacks connecting remote sea surface temperature changes (SST anomalies) to local soil moisture and boundary layer responses. Seasonal and Agricultural droughts are particularly useful test beds for examining these feedback processes because they are typically characterized by prolonged stretches of rain-free days followed by some termination condition. To quantify the full process-chain across these distinct spatial scales, complimentary information from several well-established land-atmosphere coupling metrics are used including, but not limited to, Mixing Diagram approaches, Soil Moisture Memory, and the Heated Condensation Framework. Preliminary analysis shows that there may be transitions from negative and positive soil moisture-atmosphere feedbacks as droughts develop. This is largely instigated by persistent atmospheric forcing that initially promotes increased surface latent heat flux, which limits boundary layer depth and dry air entrainment. However, if stagnant synoptic conditions continue eventually soil moisture is depleted to the point of shutting off surface latent heat flux producing deep boundary layers and increased dry air entrainment thus deepening drought stress. A package of standardized Fortran 90 modules called the Coupling Metrics Toolkit (CoMeT; https://github.com/abtawfik/coupling-metrics) used to calculate these land-atmosphere coupling metrics is also briefly presented.

Effect of Global Warming and Increased Freshwater Flux on Northern Hemispheric Cooling

NASA Astrophysics Data System (ADS)

Girihagama, L. N.; Nof, D.

2016-02-01

We wish to answer the, fairly complicated, question of whether global warming and an increased freshwater flux can cause Northern Hemispheric warming or cooling. Starting from the assumption that the ocean is the primary source of variability in the Northern hemispheric ocean-atmosphere coupled system, we employed a simple non-linear one-dimensional coupled ocean-atmosphere model. The simplicity of the model allows us to analytically predict the evolution of many dynamical variables of interest such as, the strength of the Atlantic Meridional overturning circulation (AMOC), temperatures of the ocean and atmosphere, mass transports, salinity, and ocean-atmosphere heat fluxes. The model results show that a reduced AMOC transport due to an increased freshwater flux causes cooling in both the atmosphere and ocean in the North Atlantic (NA) deep-water formation region. Cooling in both the ocean and atmosphere can cause reduction of the ocean-atmosphere temperature difference, which in turn reduces heat fluxes in both the ocean and atmosphere. For present day climate parameters, the calculated critical freshwater flux needed to arrest AMOC is 0.08 Sv. For a constant atmospheric zonal flow, there is minimal reduction in the AMOC strength, as well as minimal warming of the ocean and atmosphere. This model provides a conceptual framework for a dynamically sound response of the ocean and atmosphere to AMOC variability as a function of increased freshwater flux. The results are qualitatively consistent with numerous realistic coupled numerical models of varying complexity.

Uncertainties and coupled error covariances in the CERA-20C, ECMWF's first coupled reanalysis ensemble

NASA Astrophysics Data System (ADS)

Feng, Xiangbo; Haines, Keith

2017-04-01

ECMWF has produced its first ensemble ocean-atmosphere coupled reanalysis, the 20th century Coupled ECMWF ReAnalysis (CERA-20C), with 10 ensemble members at 3-hour resolution. Here the analysis uncertainties (ensemble spread) of lower atmospheric variables and sea surface temperature (SST), and their correlations, are quantified on diurnal, seasonal and longer timescales. The 2-m air temperature (T2m) spread is always larger than the SST spread at high-frequencies, but smaller on monthly timescales, except in deep convection areas, indicating increasing SST control at longer timescales. Spatially the T2m-SST ensemble correlations are the strongest where ocean mixed layers are shallow and can respond to atmospheric variability. Where atmospheric convection is strong with a deep precipitating boundary layer, T2m-SST correlations are greatly reduced. As the 20th-century progresses more observations become available, and ensemble spreads decline at all variability timescales. The T2m-SST correlations increase through the 20th-century, except in the tropics. As winds become better constrained over the oceans with less spread, T2m-SST become more correlated. In the tropics, strong ENSO-related inter-annual variability is found in the correlations, as atmospheric convection centres move. These ensemble spreads have been used to provide background errors for the assimilation throughout the reanalysis, have implications for the weights given to observations, and are a general measure of the uncertainties in the analysed product. Although cross boundary covariances are not currently used, they offer considerable potential for strengthening the ocean-atmosphere coupling in future reanalyses.

Development and verification of a new wind speed forecasting system using an ensemble Kalman filter data assimilation technique in a fully coupled hydrologic and atmospheric model

NASA Astrophysics Data System (ADS)

Williams, John L.; Maxwell, Reed M.; Monache, Luca Delle

2013-12-01

Wind power is rapidly gaining prominence as a major source of renewable energy. Harnessing this promising energy source is challenging because of the chaotic nature of wind and its inherently intermittent nature. Accurate forecasting tools are critical to support the integration of wind energy into power grids and to maximize its impact on renewable energy portfolios. We have adapted the Data Assimilation Research Testbed (DART), a community software facility which includes the ensemble Kalman filter (EnKF) algorithm, to expand our capability to use observational data to improve forecasts produced with a fully coupled hydrologic and atmospheric modeling system, the ParFlow (PF) hydrologic model and the Weather Research and Forecasting (WRF) mesoscale atmospheric model, coupled via mass and energy fluxes across the land surface, and resulting in the PF.WRF model. Numerous studies have shown that soil moisture distribution and land surface vegetative processes profoundly influence atmospheric boundary layer development and weather processes on local and regional scales. We have used the PF.WRF model to explore the connections between the land surface and the atmosphere in terms of land surface energy flux partitioning and coupled variable fields including hydraulic conductivity, soil moisture, and wind speed and demonstrated that reductions in uncertainty in these coupled fields realized through assimilation of soil moisture observations propagate through the hydrologic and atmospheric system. The sensitivities found in this study will enable further studies to optimize observation strategies to maximize the utility of the PF.WRF-DART forecasting system.

Direct-Coupled Plasma-Assisted Combustion Using a Microwave Waveguide Torch

DTIC Science & Technology

2011-12-01

enhance combustion by coupling an atmospheric plasma dis- charge to a premixed methane/air flame. The absorbed microwave power ranges from 60 to 150 W...The plasma system allows for complete access of the plasma- enhanced flame for laser and optical diagnostics 0093-3813/$26.00 © 2011 IEEE Report...microwave waveguide is used to initiate and enhance combustion by coupling an atmospheric plasma discharge to a premixed methane/air flame. The

A numerical study of the effect of irrigation on land-atmosphere interactions in a spring wheat cropland in India using a coupled atmosphere-crop growth dynamics model

NASA Astrophysics Data System (ADS)

Kumari, S.; Sharma, P.; Srivastava, A.; Rastogi, D.; Sehgal, V. K.; Dhakar, R.; Roy, S. B.

2017-12-01

Vegetation dynamics and surface meteorology are tightly coupled through the exchange of momentum, moisture and heat between the land surface and the atmosphere. In this study, we use a recently developed coupled atmosphere-crop growth dynamics model to study these exchanges and their effects in a spring wheat cropland in northern India. In particular, we investigate the role of irrigation in controlling crop growth rates, surface meteorology, and sensible and latent heat fluxes. The model is developed by implementing a crop growth module based on the Simple and Universal Crop growth Simulator (SUCROS) model in the Weather Research Forecasting (WRF) mesoscale atmospheric model. The crop module calculates photosynthesis rates, carbon assimilation, and biomass partitioning as a function of environmental factors and crop development stage. The leaf area index (LAI) and root depth calculated by the crop module is then fed to the Noah-MP land module of WRF to calculate land-atmosphere fluxes. The crop model is calibrated using data from an experimental spring wheat crop site in the Indian Agriculture Research Institute. The coupled model is capable of simulating the observed spring wheat phenology. Irrigation is simulated by changing the soil moisture levels from 50% - 100% of field capacity. Results show that the yield first increases with increasing soil moisture and then starts decreasing as we further increase the soil moisture. Yield attains its maximum value with soil moisture at the level of 60% water of FC. At this level, high LAI values lead to a decrease in the Bowen Ratio because more energy is transferred to the atmosphere as latent heat rather than sensible heat resulting in a cooling effect on near-surface air temperatures. Apart from improving simulation of land-atmosphere interactions, this coupled modeling approach can form the basis for the seamless crop yield and seasonal scale weather outlook prediction system.

Altitude release mechanism

DOEpatents

Kulhanek, Frank C.

1977-01-01

An altitude release mechanism for releasing a radiosonde or other measuring instrument from a balloon carrying it up into the atmosphere includes a bottle partially filled with water, a tube sealed into the bottle having one end submerged in the water in the bottle and the free end extending above the top of the bottle and a strip of water-disintegrable paper held within the free end of the tube linking the balloon to the remainder of the package. As the balloon ascends, the lowered atmospheric air pressure causes the air in the bottle to expand, forcing the water in the bottle up the tubing to wet and disintegrate the paper, releasing the package from the balloon.

Making Mars habitable

NASA Technical Reports Server (NTRS)

Mckay, Christopher P.; Toon, Owen B.; Kasting, James F.

1991-01-01

The possibility is considered that the atmosphere and climate of Mars could be altered to allow terrestrial life forms, and possibly human beings, to survive on the surface. Production of CFCs or other greenhouse gases on Mars would warm the surface enough for the regolith and polar caps to release their CO2 and raise atmospheric pressure to 100 mbar. If a large regolith and polar CO2 reservoirs exist, the pressure would continue to rise on its own. If these are absent, additional CO2 would have to be released from carbonate minerals. At this point, perhaps between 100 and 100,000 yrs, Mars might be suitable for plants. If there is a mechanism for sequestering the reduced carbon, these plants could slowly transform the CO2 to produce an O2-rich atmosphere in perhaps 100,000 yrs. If sufficient N2 could be released from putative soil deposits and the CO2 level could be kept low enough, then a human-breathable atmosphere would be produced.

Mechanical energy storage device for hip disarticulation

NASA Technical Reports Server (NTRS)

Vallotton, W. C. (Inventor)

1977-01-01

An artificial leg including a trunk socket, a thigh section hingedly coupled to the trunk socket, a leg section hingedly coupled to the thigh section and a foot section hingedly coupled to the leg section is outlined. A mechanical energy storage device is operatively associated with the artificial leg for storage and release of energy during the normal walking stride of the user. Energy is stored in the mechanical energy storage device during a weight-bearing phase of the walking stride when the user's weight is on the artificial leg. Energy is released during a phase of the normal walking stride, when the user's weight is removed from the artificial leg. The stored energy is released from the energy storage device to pivot the thigh section forwardly about the hinged coupling to the trunk socket.

Assimilating concentration observations for transport and dispersion modeling in a meandering wind field

NASA Astrophysics Data System (ADS)

Haupt, Sue Ellen; Beyer-Lout, Anke; Long, Kerrie J.; Young, George S.

Assimilating concentration data into an atmospheric transport and dispersion model can provide information to improve downwind concentration forecasts. The forecast model is typically a one-way coupled set of equations: the meteorological equations impact the concentration, but the concentration does not generally affect the meteorological field. Thus, indirect methods of using concentration data to influence the meteorological variables are required. The problem studied here involves a simple wind field forcing Gaussian dispersion. Two methods of assimilating concentration data to infer the wind direction are demonstrated. The first method is Lagrangian in nature and treats the puff as an entity using feature extraction coupled with nudging. The second method is an Eulerian field approach akin to traditional variational approaches, but minimizes the error by using a genetic algorithm (GA) to directly optimize the match between observations and predictions. Both methods show success at inferring the wind field. The GA-variational method, however, is more accurate but requires more computational time. Dynamic assimilation of a continuous release modeled by a Gaussian plume is also demonstrated using the genetic algorithm approach.

Gas chromatography coupled to atmospheric pressure ionization mass spectrometry (GC-API-MS): review.

PubMed

Li, Du-Xin; Gan, Lin; Bronja, Amela; Schmitz, Oliver J

2015-09-03

Although the coupling of GC/MS with atmospheric pressure ionization (API) has been reported in 1970s, the interest in coupling GC with atmospheric pressure ion source was expanded in the last decade. The demand of a "soft" ion source for preserving highly diagnostic molecular ion is desirable, as compared to the "hard" ionization technique such as electron ionization (EI) in traditional GC/MS, which fragments the molecule in an extensive way. These API sources include atmospheric pressure chemical ionization (APCI), atmospheric pressure photoionization (APPI), atmospheric pressure laser ionization (APLI), electrospray ionization (ESI) and low temperature plasma (LTP). This review discusses the advantages and drawbacks of this analytical platform. After an introduction in atmospheric pressure ionization the review gives an overview about the history and explains the mechanisms of various atmospheric pressure ionization techniques used in combination with GC such as APCI, APPI, APLI, ESI and LTP. Also new developments made in ion source geometry, ion source miniaturization and multipurpose ion source constructions are discussed and a comparison between GC-FID, GC-EI-MS and GC-API-MS shows the advantages and drawbacks of these techniques. The review ends with an overview of applications realized with GC-API-MS. Copyright © 2015. Published by Elsevier B.V.

Volcanic Gas

MedlinePlus

... and pressure decreases, gases are released from the liquid portion of the magma (melt) and continue to travel upward and are eventually released into the atmosphere. Large eruptions can release enormous amounts of gas in a short time. The 1991 eruption of ...

Greenhouse gas emissions from oilfield-produced water in Shengli Oilfield, Eastern China.

PubMed

Yang, Shuang; Yang, Wei; Chen, Guojun; Fang, Xuan; Lv, Chengfu; Zhong, Jiaai; Xue, Lianhua

2016-08-01

Greenhouse gas (GHG) emissions from oil and gas systems are an important component of the GHG emission inventory. To assess the carbon emissions from oilfield-produced water under atmospheric conditions correctly, in situ detection and simulation experiments were developed to study the natural release of GHG into the atmosphere in the Shengli Oilfield, the second largest oilfield in China. The results showed that methane (CH4) and carbon dioxide (CO2) were the primary gases released naturally from the oilfield-produced water. The atmospheric temperature and release time played important roles in determining the CH4 and CO2 emissions under atmospheric conditions. Higher temperatures enhanced the carbon emissions. The emissions of both CH4 and CO2 from oilfield-produced water were highest at 27°C and lowest at 3°C. The bulk of CH4 and CO2 was released from the oilfield-produced water during the first release period, 0-2hr, for each temperature, with a maximum average emission rate of 0.415gCH4/(m(3)·hr) and 3.934gCO2/(m(3)·hr), respectively. Then the carbon emissions at other time periods gradually decreased with the extension of time. The higher solubility of CO2 in water than CH4 results in a higher emission rate of CH4 than CO2 over the same release duration. The simulation proved that oilfield-produced water is one of the potential emission sources that should be given great attention in oil and gas systems. Copyright © 2016. Published by Elsevier B.V.

Venusian Earthquakes Detection by Ionospheric Sounding

NASA Astrophysics Data System (ADS)

Occhipinti, G.; Lognonne, P.; Garcia, R. F.; Gudkova, T.

2010-12-01

Thanks to technological advances over the past fifteen years the ionosphere is now a new medium for seismological investigation. As a consequence of density structure in Venus atmosphere, the coupling between solid and fluid part of Venus induce a more significant atmospheric responce to quakes and volcanic eruptions (Lognonné & Johnson, 2007). Equivalent perturbation induced by internal activity has been detected on Earth through their subsequent ionospheric signature imaged by ionospheric tools (Doppler sounding or GPS) (Lognonné et al., 2006, Occhipinti et al., 2010). The strong solid/atmosphere coupling on Venus (Garcia et al., 2005, 2009), the thin ionospheric layer as well as absence of magnetic field present optimal circumstances for a better detection of these signals on Venus than on Earth. Consequently, ionospheric Doppler sounders on-board orbiters or balloons will provide informations on the infrasonic response of the atmosphere/ionosphere to quakes, and will help to constrain the interior structure of Venus through the solid/atmosphere coupling. With this paper we explore the future mission possibility and constrains.

Solar variability, coupling between atmospheric layers and climate change.

PubMed

Arnold, Neil

2002-12-15

One of the enduring puzzles of atmospheric physics is the extent to which changes in the Sun can influence the behaviour of the climate system. While solar-flux changes tend to be relatively modest, a number of observations of atmospheric parameters indicates a disproportionately large response. Global-scale models of the coupled middle and upper atmosphere have provided new insights into some of the mechanisms that may be responsible for the amplification of the solar signal. In particular, modification of the transport of heat and chemicals such as ozone by waves during periods of solar activity has been shown to make an important contribution to the climate of the stratosphere and mesosphere. In this paper, a review of some of the recent advances in understanding the coupling between atmospheric layers and how this work relates to Sun-weather relations and climate change in the troposphere will be presented, along with a discussion of some of the challenges that remain.

Diagnosing the Nature of Land-Atmosphere Coupling During the 2006-7 Dry/Wet Extremes in the U.S. Southern Great Plains

NASA Technical Reports Server (NTRS)

Santanello, Joseph A., Jr.; Peters-Lidard, Christa D.; Kumar, Sujay V.; Dong, Xiquan; Kennedy, Aaron D.

2011-01-01

Land-atmosphere interactions play a critical role in determining the. diurnal evolution of both planetary boundary layer (PBL) and land surface temperature and moisture states. The degree of coupling between the land surface and PBL in numerical weather prediction and climate models remains largely unexplored and undiagnosed due to the complex interactions and feedbacks present across a range of scales. Further, uncoupled systems or experiments (e.g., the Project for Intercomparison of Land Parameterization Schemes, PILPS) may lead to inaccurate water and energy cycle process understanding by neglecting feedback processes such as PBL-top entrainment. In this study, a framework for diagnosing local land-atmosphere coupling (LoCo) is presented using a coupled mesoscale model with a suite of PBL and land surface model (LSM) options along with observations during the summers of 200617 in the U.S. Southern Great Plains. Specifically, the Weather Research and Forecasting (WRF) model has been coupled to NASA's Land Information System (LIS), which provides a flexible and high-resolution representation and initialization of land surface physics and states. A range of diagnostics exploring the links and feedbacks between soil moisture and precipitation are examined for the dry/wet extremes of this region, along with the sensitivity of PBL-LSM coupling to perturbations in soil moisture. As such, this methodology provides a potential pathway to study factors controlling local land-atmosphere coupling (LoCo) using the LIS-WRF system, which is serving as a testbed for LoCo experiments to evaluate coupling diagnostics within the community.

Impact of vegetation on land-atmosphere coupling strength and its implication for desertification mitigation over East Asia

NASA Astrophysics Data System (ADS)

Myoung, Boksoon; Choi, Yong-Sang; Choi, Suk-Jin; Park, Seon Ki

2012-06-01

Desertification of the East Asian drylands and the consequent dust transport have been serious concerns for adjacent Asian countries as well as the western United States. Tree planting has been considered one applicable strategy to mitigate the desertification. However, the desired effect of the tree planting would not be brought to fruition unless the newly planted trees change the coupling characteristics between the land and the atmosphere. Based on this perception, we attempt to clarify the effects of vegetation on the coupling strength between the atmosphere and land surface, and we suggest the most efficient areas of tree planting for desertification mitigation in East Asia. Using regional vegetation-atmosphere coupled model simulations, coupling strength with and without vegetation was computed and compared with each other. An increased vegetation fraction reduces the coupling strength in June, July, and August (JJA), primarily due to decreased evapotranspiration variability. This effect is pronounced over the Manchurian Plains and the highly populated areas of Beijing and Tianjin. The reduced coupling strength tends to weaken feedback between soil moisture and precipitation as a maintenance mechanism of warm season droughts in the midlatitudes and subsequently decrease the probability of droughts, a finding that is reflected in the enhanced JJA mean soil moisture. However, some drylands like the eastern edges of the Gobi desert present marginal or even opposite changes in coupling strength, meaning a limited effect of vegetation on relieving droughts. Therefore, given limited financial and human resources, acupuncture-like afforestation, i.e., concentrated tree planting in a particular region where the coupling strength can be substantially reduced by vegetation, is an effective strategy to secure long-standing desertification mitigation.

Modeling and Observational Framework for Diagnosing Local Land-Atmosphere Coupling on Diurnal Time Scales

NASA Technical Reports Server (NTRS)

Santanello, Joseph A., Jr.; Peters-Lidard, Christa D.; Kumar, Sujay V.; Alonge, Charles; Tao, Wei-Kuo

2009-01-01

Land-atmosphere interactions play a critical role in determining the diurnal evolution of both planetary boundary layer (PBL) and land surface temperature and moisture states. The degree of coupling between the land surface and PBL in numerical weather prediction and climate models remains largely unexplored and undiagnosed due to the complex interactions and feedbacks present across a range of scales. Further, uncoupled systems or experiments (e.g., the Project for Intercomparison of Land Parameterization Schemes, PILPS) may lead to inaccurate water and energy cycle process understanding by neglecting feedback processes such as PBL-top entrainment. In this study, a framework for diagnosing local land-atmosphere coupling is presented using a coupled mesoscale model with a suite of PBL and land surface model (LSM) options along with observations during field experiments in the U. S. Southern Great Plains. Specifically, the Weather Research and Forecasting (WRF) model has been coupled to the Land Information System (LIS), which provides a flexible and high-resolution representation and initialization of land surface physics and states. Within this framework, the coupling established by each pairing of the available PBL schemes in WRF with the LSMs in LIS is evaluated in terms of the diurnal temperature and humidity evolution in the mixed layer. The co-evolution of these variables and the convective PBL is sensitive to and, in fact, integrative of the dominant processes that govern the PBL budget, which are synthesized through the use of mixing diagrams. Results show how the sensitivity of land-atmosphere interactions to the specific choice of PBL scheme and LSM varies across surface moisture regimes and can be quantified and evaluated against observations. As such, this methodology provides a potential pathway to study factors controlling local land-atmosphere coupling (LoCo) using the LIS-WRF system, which will serve as a testbed for future experiments to evaluate coupling diagnostics within the community.

Magnetosphere - Ionosphere - Thermosphere (MIT) Coupling at Jupiter

NASA Astrophysics Data System (ADS)

Yates, J. N.; Ray, L. C.; Achilleos, N.

2017-12-01

Jupiter's upper atmospheric temperature is considerably higher than that predicted by Solar Extreme Ultraviolet (EUV) heating alone. Simulations incorporating magnetosphere-ionosphere coupling effects into general circulation models have, to date, struggled to reproduce the observed atmospheric temperatures under simplifying assumptions such as azimuthal symmetry and a spin-aligned dipole magnetic field. Here we present the development of a full three-dimensional thermosphere model coupled in both hemispheres to an axisymmetric magnetosphere model. This new coupled model is based on the two-dimensional MIT model presented in Yates et al., 2014. This coupled model is a critical step towards to the development of a fully coupled 3D MIT model. We discuss and compare the resulting thermospheric flows, energy balance and MI coupling currents to those presented in previous 2D MIT models.

Study of the Effect of Wind Speed on Evaporation from Soil Through Integrated Modeling of Atmospheric Boundary Layer and Shallow Subsurface

NASA Astrophysics Data System (ADS)

Smits, K. M.; Davarzani, H.; Illangasekare, T. H.

2012-12-01

The study of the interaction between the land and atmosphere is paramount to our understanding of many emerging problems to include climate change and the movement of green house gases such as possible leaking of sequestered CO2. Soil moisture distribution in the shallow subsurface becomes a critical factor in these problems. The heat and mass flux in the form of soil evaporation across the land surface couples the atmospheric boundary layer to the shallow subsurface. The coupling between land and the atmosphere leads to highly dynamic interactions between the porous media properties, transport processes and boundary conditions, resulting in dynamic evaporative behavior. However, the coupling at the land-atmospheric interface is rarely considered in most current models and their validation for practical applications. This is due to the complexity of the problem in field scenarios and the scarcity of field or laboratory data capable of testing and refining coupled energy and mass transfer theories. In most efforts to compute evaporation from soil, only indirect coupling is provided to characterize the interaction between non-isothermal multiphase flows under realistic atmospheric conditions even though heat and mass flux are controlled by the coupled dynamics of the land and the atmospheric boundary layer. In earlier drying modeling concepts, imposing evaporation flux (kinetic of relative humidity) and temperature as surface boundary condition is often needed. With the goal of improving our understanding of the land/atmospheric coupling, we developed a model based on the coupling of Navier-Stokes free flow and Darcy flow in porous medium. The model consists of the coupled equations of mass conservation for the liquid phase (water) and gas phase (water vapor and air) in porous medium with gas phase (water vapor and air) in free flow domain under non-isothermal, non-equilibrium conditions. The boundary conditions at the porous medium-free flow medium interface include dynamical, thermal and solutal equilibriums, and using the Beavers-Joseph slip boundary condition. What is unique about this model is that the evaporation rate and soil surface temperature conditions come directly from the model output. In order to experimentally validate the numerical results, we developed and used a unique two dimensional wind tunnel placed above a soil tank equipped with a network of different sensors. A series of experiments under varying boundary conditions were performed. Precision data under well-controlled transient heat and wind boundary conditions was generated. Results from numerical simulations were compared with experimental data. Results demonstrate that the coupling concept can predict the different stages of the drying process in porous media with good accuracy. Increasing the wind speed increases the first stage evaporation rate and decreases the transition time at low velocity values; then, at high values of wind speed the evaporation rate becomes less dependent of flow in free fluid. In the opposite, the impact of the wind speed on the second stage evaporation (diffusion dominant stage) is not significant. The proposed theoretical model can be used to predict the evaporation process where a porous medium flow is coupled to a free flow for different practical applications.

Framework of distributed coupled atmosphere-ocean-wave modeling system

NASA Astrophysics Data System (ADS)

Wen, Yuanqiao; Huang, Liwen; Deng, Jian; Zhang, Jinfeng; Wang, Sisi; Wang, Lijun

2006-05-01

In order to research the interactions between the atmosphere and ocean as well as their important role in the intensive weather systems of coastal areas, and to improve the forecasting ability of the hazardous weather processes of coastal areas, a coupled atmosphere-ocean-wave modeling system has been developed. The agent-based environment framework for linking models allows flexible and dynamic information exchange between models. For the purpose of flexibility, portability and scalability, the framework of the whole system takes a multi-layer architecture that includes a user interface layer, computational layer and service-enabling layer. The numerical experiment presented in this paper demonstrates the performance of the distributed coupled modeling system.

Coupled Data Assimilation in Navy ESPC

NASA Astrophysics Data System (ADS)

Barron, C. N.; Spence, P. L.; Frolov, S.; Rowley, C. D.; Bishop, C. H.; Wei, M.; Ruston, B.; Smedstad, O. M.

2017-12-01

Data assimilation under global coupled Earth System Prediction Capability (ESPC) presents significantly greater challenges than data assimilation in forecast models of a single earth system like the ocean and atmosphere. In forecasts of a single component, data assimilation has broad flexibility in adjusting boundary conditions to reduce forecast errors; coupled ESPC requires consistent simultaneous adjustment of multiple components within the earth system: air, ocean, ice, and others. Data assimilation uses error covariances to express how to consistently adjust model conditions in response to differences between forecasts and observations; in coupled ESPC, these covariances must extend from air to ice to ocean such that changes within one fluid are appropriately balanced with corresponding adjustments in the other components. We show several algorithmic solutions that allow us to resolve these challenges. Specifically, we introduce the interface solver method that augments existing stand-alone systems for ocean and atmosphere by allowing them to be influenced by relevant measurements from the coupled fluid. Plans are outlined for implementing coupled data assimilation within ESPC for the Navy's global coupled model. Preliminary results show the impact of assimilating SST-sensitive radiances in the atmospheric model and first results of hybrid DA in a 1/12 degree model of the global ocean.

An equilibrium model for the coupled ocean-atmosphere boundary layer in the tropics

NASA Technical Reports Server (NTRS)

Sui, C.-H.; Lau, K.-M.; Betts, Alan K.

1991-01-01

An atmospheric convective boundary layer (CBL) model is coupled to an ocean mixed-layer (OML) model in order to study the equilibrium state of the coupled system in the tropics, particularly in the Pacific region. The equilibrium state of the coupled system is solved as a function of sea-surface temperature (SST) for a given surface wind and as a function of surface wind for a given SST. It is noted that in both cases, the depth of the CBL and OML increases and the upwelling below the OML decreases, corresponding to either increasing SST or increasing surface wind. The coupled ocean-atmosphere model is solved iteratively as a function of surface wind for a fixed upwelling and a fixed OML depth, and it is observed that SST falls with increasing wind in both cases. Realistic gradients of mixed-layer depth and upwelling are observed in experiments with surface wind and SST prescribed as a function of longitude.

Oxygen cycling in the northern Benguela Upwelling System: Modelling oxygen sources and sinks

NASA Astrophysics Data System (ADS)

Schmidt, Martin; Eggert, Anja

2016-12-01

This paper elucidates the oxygen dynamics in the northern Benguela Upwelling System by means of process oriented, numerical modelling. Owing to the complex physical-biological interaction in this system, a coupled hydrodynamic-biogeochemical model is required to grasp the various aspects of the oxygen dynamics. We used high-resolution atmospheric fields derived from observations to force our model, available since 1999. The model results represent a 15 years, consistent data set of realistic hydrographic and ecosystem variables, including oxygen distribution patterns. After a concise description of the main aspects of the model, we use the model data to analyse the components contributing to the oxygen dynamics, namely, the ocean circulation, the exchange between ocean and atmosphere as well as the local biogeochemical oxygen cycling in the system. We thoroughly validate the model with available field observations and remote sensing data. The strengths of coastal upwelling, which controls the nutrient supply to the euphotic zone, as well as the poleward undercurrent that carries oxygen and nutrients to the shelf in the northern Benguela Upwelling System are well reproduced in the model. Among the biological oxygen sinks, mineralisation in the sediment, respiration of zooplankton and nitrification in the water column are important. We also found that vertical migration of zooplankton in response to the oxygen conditions provides a regulating feedback, which may prevent a complete deoxygenation of suboxic waters. As long as oxygen or nitrate are available in the bottom waters, the activities of chemolithoautotrophic sulphur bacteria on the sediment surface keep the redoxcline within the sediment and prevent the release of hydrogen sulphide into the water column. By horizontal integration of the simulated ocean-atmosphere oxygen flux, it can be shown that the Kunene upwelling cell between 16 ° S and 18 ° S is a boundary between the equatorial ocean, characterise by weak oxygen release to the atmosphere, and the subtropical Benguela Upwelling System governed by an enhanced and seasonal varying flux. Furthermore, a comparison of oxygen fluxes controlled by physical transport versus biogeochemical processes shows that the physical processes dominate in the northern Benguela Upwelling System.

Atmospheric and Space Sciences: Ionospheres and Plasma Environments

NASA Astrophysics Data System (ADS)

Yiǧit, Erdal

2018-01-01

The SpringerBriefs on Atmospheric and Space Sciences in two volumes presents a concise and interdisciplinary introduction to the basic theory, observation & modeling of atmospheric and ionospheric coupling processes on Earth. The goal is to contribute toward bridging the gap between meteorology, aeronomy, and planetary science. In addition recent progress in several related research topics, such atmospheric wave coupling and variability, is discussed. Volume 1 will focus on the atmosphere, while Volume 2 will present the ionospheres and the plasma environments. Volume 2 is aimed primarily at (research) students and young researchers that would like to gain quick insight into the basics of space sciences and current research. In combination with the first volume, it also is a useful tool for professors who would like to develop a course in atmospheric and space physics.

Ion Release and Galvanic Corrosion of Different Orthodontic Brackets and Wires in Artificial Saliva.

PubMed

Tahmasbi, Soodeh; Sheikh, Tahereh; Hemmati, Yasamin B

2017-03-01

To investigate the galvanic corrosion of brackets manufactured by four different companies coupled with stainless steel (SS) or nickel-titanium (NiTi) wires in an artificial saliva solution. A total of 24 mandibular central incisor Roth brackets of four different manufacturers (American Orthodontics, Dentaurum, Shinye, ORJ) were used in this experimental study. These brackets were immersed in artificial saliva along with SS or NiTi orthodontic wires (0.016'', round) for 28 days. The electric potential difference of each bracket/ wire coupled with a saturated calomel reference electrode was measured via a voltmeter and recorded constantly. Corrosion rate (CR) was calculated, and release of ions was measured with an atomic absorption spectrometer. Stereomicroscope was used to evaluate all samples. Then, samples with corrosion were further assessed by scanning electron microscope and energy-dispersive X-ray spectroscopy. Two-way analysis of variance was used to analyze data. Among ions evaluated, release of nickel ions from Shinye brackets was significantly higher than that of other brackets. The mean potential difference was significantly lower in specimens containing a couple of Shinye brackets and SS wire compared with other specimens. No significant difference was observed in the mean CR of various groups (p > 0.05). Microscopic evaluation showed corrosion in two samples only: Shinye bracket coupled with SS wire and American Orthodontics bracket coupled with NiTi wire. Shinye brackets coupled with SS wire showed more susceptibility to galvanic corrosion. There were no significant differences among specimens in terms of the CR or released ions except the release of Ni ions, which was higher in Shinye brackets.

Modelling of auroral electrodynamical processes: Magnetosphere to mesosphere

NASA Technical Reports Server (NTRS)

Chiu, Y. T.; Gorney, D. J.; Kishi, A. M.; Newman, A. L.; Schulz, M.; Walterscheid, R. L.; CORNWALL; Prasad, S. S.

1982-01-01

Research conducted on auroral electrodynamic coupling between the magnetosphere and ionosphere-atmosphere in support of the development of a global scale kinetic plasma theory is reviewed. Topics covered include electric potential structure in the evening sector; morning and dayside auroras; auroral plasma formation; electrodynamic coupling with the thermosphere; and auroral electron interaction with the atmosphere.

Origin of seasonal predictability for summer climate over the Northwestern Pacific

PubMed Central

Kosaka, Yu; Xie, Shang-Ping; Lau, Ngar-Cheung; Vecchi, Gabriel A.

2013-01-01

Summer climate in the Northwestern Pacific (NWP) displays large year-to-year variability, affecting densely populated Southeast and East Asia by impacting precipitation, temperature, and tropical cyclones. The Pacific–Japan (PJ) teleconnection pattern provides a crucial link of high predictability from the tropics to East Asia. Using coupled climate model experiments, we show that the PJ pattern is the atmospheric manifestation of an air–sea coupled mode spanning the Indo-NWP warm pool. The PJ pattern forces the Indian Ocean (IO) via a westward propagating atmospheric Rossby wave. In response, IO sea surface temperature feeds back and reinforces the PJ pattern via a tropospheric Kelvin wave. Ocean coupling increases both the amplitude and temporal persistence of the PJ pattern. Cross-correlation of ocean–atmospheric anomalies confirms the coupled nature of this PJIO mode. The ocean–atmosphere feedback explains why the last echoes of El Niño–Southern Oscillation are found in the IO-NWP in the form of the PJIO mode. We demonstrate that the PJIO mode is indeed highly predictable; a characteristic that can enable benefits to society. PMID:23610388

Late Coupled Evolution of Venus' Atmosphere and the Effects of Meteoritic Impacts

NASA Astrophysics Data System (ADS)

Gillmann, C.; Tackley, P. J.; Golabek, G.

2013-12-01

We investigate what mechanisms and events could have led to the divergent evolution of Venus and Earth. We propose develop our investigation of the post-magma-ocean history of the atmosphere and surface conditions on Venus through a coupled model of mantle/atmosphere evolution by including meteoritic impacts in our previous work. Our main focuses are mechanisms that deplete or replenish the atmosphere: volcanic degassing, atmospheric escape and impacts. Atmospheric escape modeling involves two different aspects. During the first few hundreds of million years, hydrodynamic escape is dominant. A significant portion of the early atmosphere can be thus removed. For later evolution, on the other hand, non-thermal escape becomes the main process as observed by the ASPERA instrument and modeled in various recent numerical studies. The atmosphere is replenished by volcanic degassing, using an adapted version of the StagYY mantle dynamics model (Armann and Tackley, 2012) and including episodic lithospheric overturn. The evolving surface temperature is calculated from CO2 and water in the atmosphere with a gray radiative-convective atmosphere model. This surface temperature in turn acts as a boundary condition for the mantle dynamics model and has an influence on the convection, volcanism and subsequent degassing. We take into account the effects of meteorites in our simulations by adapting each relevant part of the model. They can bring volatiles as well as erode the atmosphere. Mantle dynamics are modified since the impact itself can also bring large amounts of energy to the mantle. A 2D distribution of the thermal anomaly due to the impact is used and can lead to melting. Volatile evolution due to impacts (especially the large ones) is heavily debated so we test a broad range of impactor parameters (size, velocity, timing) and test different assumptions related to impact erosion going from large eroding power (Ahrens 1993) to recent parameterization (Shuvalov, 2009, 2010). We obtain a Venus-like behavior for the solid planet and atmospheric evolution leading to present-day conditions. Without any impact, CO2 pressure seems unlikely to vary much over the history of the planet, only slightly increasing due to degassing. A late build-up of the atmosphere with several resurfacing events seems unlikely. On the other hand, water pressure is strongly sensitive to volcanic activity and varies rapidly leading to variations in surface temperatures of up to 200K, which have been identified to have an effect on volcanic activity. We observe a clear correlation between low temperature and mobile lid regime. Impacts can strongly change this picture. While small (less than kilometer scale) meteorites have a negligible effect, medium ones are able to bring volatiles to the planet and generate melt both at the impact and later on, due to volcanic events they triggered due to the changes they make to mantle dynamics. A significant amount of volatiles (compared to present-day atmosphere) can be released on a short timescale, which can increase the surface temperature by tens of Kelvin. Larger impactors (~100 km) have even stronger effects as they can blow upwards of 10% of the atmosphere away, depending on the parameters. Removing more than 80% of the atmosphere on the impact is clearly feasible. In these cases, later degassing is also massive, which mitigates the volatile sink.

Decreased atmospheric sulfur deposition across the southeastern U.S.: When will watersheds release stored sulfate?

Treesearch

Karen C. Rice; Todd M. Scanlon; Jason A. Lynch; Bernard J. Cosby

2014-01-01

Emissions of sulfur dioxide (SO2) to the atmosphere lead to atmospheric deposition of sulfate (SO42-), which is the dominant strong acid anion causing acidification of surface waters and soils in the eastern United States. Since passage of the Clean Air Act and its Amendments, atmospheric deposition...

Space fireworks for upper atmospheric wind measurements by sounding rocket experiments

NASA Astrophysics Data System (ADS)

Yamamoto, M.

2016-01-01

Artificial meteor trains generated by chemical releases by using sounding rockets flown in upper atmosphere were successfully observed by multiple sites on ground and from an aircraft. We have started the rocket experiment campaign since 2007 and call it "Space fireworks" as it illuminates resonance scattering light from the released gas under sunlit/moonlit condition. By using this method, we have acquired a new technique to derive upper atmospheric wind profiles in twilight condition as well as in moonlit night and even in daytime. Magnificent artificial meteor train images with the surrounding physics and dynamics in the upper atmosphere where the meteors usually appear will be introduced by using fruitful results by the "Space firework" sounding rocket experiments in this decade.

Impacts of Atmosphere-Ocean Coupling on Southern Hemisphere Climate Change

NASA Technical Reports Server (NTRS)

Li, Feng; Newman, Paul; Pawson, Steven

2013-01-01

Climate in the Southern Hemisphere (SH) has undergone significant changes in recent decades. These changes are closely linked to the shift of the Southern Annular Mode (SAM) towards its positive polarity, which is driven primarily by Antarctic ozone depletion. There is growing evidence that Antarctic ozone depletion has significant impacts on Southern Ocean circulation change. However, it is poorly understood whether and how ocean feedback might impact the SAM and climate change in the SH atmosphere. This outstanding science question is investigated using the Goddard Earth Observing System Coupled Atmosphere-Ocean-Chemistry Climate Model(GEOS-AOCCM).We perform ensemble simulations of the recent past (1960-2010) with and without the interactive ocean. For simulations without the interactive ocean, we use sea surface temperatures and sea ice concentrations produced by the interactive ocean simulations. The differences between these two ensemble simulations quantify the effects of atmosphere-ocean coupling. We will investigate the impacts of atmosphere-ocean coupling on stratospheric processes such as Antarctic ozone depletion and Antarctic polar vortex breakup. We will address whether ocean feedback affects Rossby wave generation in the troposphere and wave propagation into the stratosphere. Another focuson this study is to assess how ocean feedback might affect the tropospheric SAM response to Antarctic ozone depletion

Verification of land-atmosphere coupling in forecast models, reanalyses and land surface models using flux site observations.

PubMed

Dirmeyer, Paul A; Chen, Liang; Wu, Jiexia; Shin, Chul-Su; Huang, Bohua; Cash, Benjamin A; Bosilovich, Michael G; Mahanama, Sarith; Koster, Randal D; Santanello, Joseph A; Ek, Michael B; Balsamo, Gianpaolo; Dutra, Emanuel; Lawrence, D M

2018-02-01

We confront four model systems in three configurations (LSM, LSM+GCM, and reanalysis) with global flux tower observations to validate states, surface fluxes, and coupling indices between land and atmosphere. Models clearly under-represent the feedback of surface fluxes on boundary layer properties (the atmospheric leg of land-atmosphere coupling), and may over-represent the connection between soil moisture and surface fluxes (the terrestrial leg). Models generally under-represent spatial and temporal variability relative to observations, which is at least partially an artifact of the differences in spatial scale between model grid boxes and flux tower footprints. All models bias high in near-surface humidity and downward shortwave radiation, struggle to represent precipitation accurately, and show serious problems in reproducing surface albedos. These errors create challenges for models to partition surface energy properly and errors are traceable through the surface energy and water cycles. The spatial distribution of the amplitude and phase of annual cycles (first harmonic) are generally well reproduced, but the biases in means tend to reflect in these amplitudes. Interannual variability is also a challenge for models to reproduce. Our analysis illuminates targets for coupled land-atmosphere model development, as well as the value of long-term globally-distributed observational monitoring.

ATMOSPHERIC RELEASES OF HEXAVALENT CHROMIUM FROM HARD CHROMIUM PLATING OPERATIONS

EPA Science Inventory

The University of Central Florida Department of Civil and Environmental Engineering is investigating methods for improved estimation of chemical releases which require reporting under provisions of SARA Title III (Toxic Release Inventory, Form R). This paper describes results fr...

Local Integration of the National Atmospheric Release Advisory Center with Cities (LINC)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ermak, D L; Tull, J E; Mosley-Rovi, R

The objective of the ''Local Integration of the National Atmospheric Release Advisory Center with Cities'' (LINC) program is to demonstrate the capability for providing local government agencies with an advanced operational atmospheric plume prediction capability, which can be seamlessly integrated with appropriate federal agency support for homeland security applications. LINC is a Domestic Demonstration and Application Program (DDAP) funded by the Chemical and Biological National Security Program (CBNP), which is part of the Department of Energy's (DOE) National Nuclear Security Administration (NNSA). LINC will make use of capabilities that have been developed the CBNP, and integrated into the National Atmosphericmore » Release Advisory Center (NARAC) at Lawrence Livermore National Laboratory (LLNL). NARAC tools services will be provided to pilot study cities and counties to map plumes from terrorism threats. Support to these local agencies will include training and customized support for exercises, special events, and general emergencies. NARAC provides tools and services that map the probable spread of hazardous material which have been accidentally or intentionally released into the atmosphere. Primarily supported by the DOE, NARAC is a national support and resource center for planning, real-time assessment and detailed studies of incidents involving a wide variety of hazards, including radiological, chemical, or biological releases. NARAC is a distributed system, providing modeling and geographical information tools for use on an end user's computer system, as well as real-time access to global meteorological and geographical databases and advanced three-dimensional model predictions.« less

Impacts of a massive release of methane and hydrogen sulfide on oxygen and ozone during the late Permian mass extinction

NASA Astrophysics Data System (ADS)

Kaiho, Kunio; Koga, Seizi

2013-08-01

The largest mass extinction of animals and plants in both the ocean and on land occurred in the late Permian (252 Ma), largely coinciding with the largest flood basalt volcanism event in Siberia and an oceanic anoxic/euxinic event. We investigated the impacts of a massive release of methane (CH4) from the Siberian igneous province and the ocean and/or hydrogen sulfide (H2S) from the euxinic ocean on oxygen and ozone using photochemical model calculations. Our calculations indicated that an approximate of 14% decrease in atmospheric O2 levels would have occurred in the case of a large combined CH4 and H2S flux to the atmosphere, whereas an approximate of 8 to 10% decrease would have occurred from the CH4 flux and oxidation of all H2S in the ocean. The slight decrease in atmospheric O2 levels may have contributed to the extinction event. We demonstrate for the first time that a massive release of CH4 from the Siberian igneous province and a coincident massive release of CH4 and H2S did not cause ozone collapse. A collapse of stratospheric ozone leading to an increase in UV is not supported by the maximum model input levels for CH4 and H2S. These conclusions on O2 and O3 are correspondent to every H2S release percentages from the ocean to the atmosphere.

Atmospheric Modeling of Mars Methane Plumes

NASA Astrophysics Data System (ADS)

Mischna, Michael A.; Allen, M.; Lee, S.

2010-10-01

We present two complementary methods for isolating and modeling surface source releases of methane in the martian atmosphere. From recent observations, there is strong evidence that periodic releases of methane occur from discrete surface locations, although the exact location and mechanism of release is still unknown. Numerical model simulations with the Mars Weather Research and Forecasting (MarsWRF) general circulation model (GCM) have been applied to the ground-based observations of atmospheric methane by Mumma et al., (2009). MarsWRF simulations reproduce the natural behavior of trace gas plumes in the martian atmosphere, and reveal the development of the plume over time. These results provide constraints on the timing and location of release of the methane plume. Additional detections of methane have been accumulated by the Planetary Fourier Spectrometer (PFS) on board Mars Express. For orbital observations, which generally have higher frequency and resolution, an alternate approach to source isolation has been developed. Drawing from the concept of natural selection within biology, we apply an evolutionary computational model to this problem of isolating source locations. Using genetic algorithms that `reward’ best-fit matches between observations and GCM plume simulations (also from MarsWRF) over many generations, we find that we can potentially isolate source locations to within tens of km, which is within the roving capabilities of future Mars rovers. Together, these methods present viable numerical approaches to restricting the timing, duration and size of methane release events, and can be used for other trace gas plumes on Mars as well as elsewhere in the solar system.

Verification and Validation of a Navy ESPC Hindcast with Loosely Coupled Data Assimilation

NASA Astrophysics Data System (ADS)

Metzger, E. J.; Barton, N. P.; Smedstad, O. M.; Ruston, B. C.; Wallcraft, A. J.; Whitcomb, T. R.; Ridout, J. A.; Franklin, D. S.; Zamudio, L.; Posey, P. G.; Reynolds, C. A.; Phelps, M.

2016-12-01

The US Navy is developing an Earth System Prediction Capability (ESPC) to provide global environmental information to meet Navy and Department of Defense (DoD) operations and planning needs from the upper atmosphere to under the sea. It will be a fully coupled global atmosphere/ocean/ice/wave/land prediction system providing daily deterministic forecasts out to 16 days at high horizontal and vertical resolution, and daily probabilistic forecasts out to 45 days at lower resolution. The system will run at the Navy DoD Supercomputing Resource Center with an initial operational capability scheduled for the end of FY18 and the final operational capability scheduled for FY22. The individual model and data assimilation components include: atmosphere - NAVy Global Environmental Model (NAVGEM) and Naval Research Laboratory (NRL) Atmospheric Variational Data Assimilation System - Accelerated Representer (NAVDAS-AR); ocean - HYbrid Coordinate Ocean Model (HYCOM) and Navy Coupled Ocean Data Assimilation (NCODA); ice - Community Ice CodE (CICE) and NCODA; WAVEWATCH III™ and NCODA; and land - NAVGEM Land Surface Model (LSM). Currently, NAVGEM/HYCOM/CICE are three-way coupled and each model component is cycling with its respective assimilation scheme. The assimilation systems do not communicate with each other, but future plans call for these to be coupled as well. NAVGEM runs with a 6-hour update cycle while HYCOM/CICE run with a 24-hour update cycle. The T359L50 NAVGEM/0.08° HYCOM/0.08° CICE system has been integrated in hindcast mode and verification/validation metrics have been computed against unassimilated observations and against stand-alone versions of NAVGEM and HYCOM/CICE. This presentation will focus on typical operational diagnostics for atmosphere, ocean, and ice analyses including 500 hPa atmospheric height anomalies, low-level winds, temperature/salinity ocean depth profiles, ocean acoustical proxies, sea ice edge, and sea ice drift. Overall, the global coupled ESPC system is performing with comparable skill to the stand-alone systems at the nowcast time.

State and Parameter Estimation for a Coupled Ocean--Atmosphere Model

NASA Astrophysics Data System (ADS)

Ghil, M.; Kondrashov, D.; Sun, C.

2006-12-01

The El-Nino/Southern-Oscillation (ENSO) dominates interannual climate variability and plays, therefore, a key role in seasonal-to-interannual prediction. Much is known by now about the main physical mechanisms that give rise to and modulate ENSO, but the values of several parameters that enter these mechanisms are an important unknown. We apply Extended Kalman Filtering (EKF) for both model state and parameter estimation in an intermediate, nonlinear, coupled ocean--atmosphere model of ENSO. The coupled model consists of an upper-ocean, reduced-gravity model of the Tropical Pacific and a steady-state atmospheric response to the sea surface temperature (SST). The model errors are assumed to be mainly in the atmospheric wind stress, and assimilated data are equatorial Pacific SSTs. Model behavior is very sensitive to two key parameters: (i) μ, the ocean-atmosphere coupling coefficient between SST and wind stress anomalies; and (ii) δs, the surface-layer coefficient. Previous work has shown that δs determines the period of the model's self-sustained oscillation, while μ measures the degree of nonlinearity. Depending on the values of these parameters, the spatio-temporal pattern of model solutions is either that of a delayed oscillator or of a westward propagating mode. Estimation of these parameters is tested first on synthetic data and allows us to recover the delayed-oscillator mode starting from model parameter values that correspond to the westward-propagating case. Assimilation of SST data from the NCEP-NCAR Reanalysis-2 shows that the parameters can vary on fairly short time scales and switch between values that approximate the two distinct modes of ENSO behavior. Rapid adjustments of these parameters occur, in particular, during strong ENSO events. Ways to apply EKF parameter estimation efficiently to state-of-the-art coupled ocean--atmosphere GCMs will be discussed.

Status and Plans for Reanalysis at NASA/GMAO

NASA Technical Reports Server (NTRS)

Gelaro, Ron

2017-01-01

Reanalysis plays a critical role in GMAOs goal to enhance NASA's program of Earth observations, providing vital data sets for climate research and the development of future missions. As the breadth of NASAs observations expands to include multiple components of the Earth system, so does the need to assimilate observations from currently uncoupled components of the system in a more physically consistent manner. GMAOs most recent reanalysis of the satellite era, MERRA-2, has completed the period 1980-present, and is now running as a continuing global climate analysis with two- to three-week latency. MERRA-2 assimilates meteorological and aerosol observations as a weakly coupled assimilation system as a first step toward GMAOs longer term goal of developing an integrated Earth system analysis (IESA) capability that will couple assimilation systems for the atmosphere, ocean, land and chemistry. The GMAO strategy is to progress incrementally toward an IESA through an evolving combination of coupled systems and offline component reanalyses driven by, for example, MERRA-2 atmospheric forcing. Most recently, the GMAO has implemented a weakly coupled assimilation scheme for analyzing ocean skin temperature within the existing atmospheric analysis. The scheme uses background fields from a near-surface ocean diurnal layer model to assimilate surface-sensitive radiances plus in-situ observations along with all other observations in the atmospheric assimilation system. In addition, MERRA-2-driven simulations of the ocean (plus sea ice) and atmospheric chemistry (for the EOS period) are currently underway, as is the development of a coupled atmosphere-ocean assimilation system. This talk will describe the status of these ongoing efforts and the planned steps toward an IESA capability for climate research.

Improving wind energy forecasts using an Ensemble Kalman Filter data assimilation technique in a fully coupled hydrologic and atmospheric model

NASA Astrophysics Data System (ADS)

Williams, J. L.; Maxwell, R. M.; Delle Monache, L.

2012-12-01

Wind power is rapidly gaining prominence as a major source of renewable energy. Harnessing this promising energy source is challenging because of the chaotic nature of wind and its propensity to change speed and direction over short time scales. Accurate forecasting tools are critical to support the integration of wind energy into power grids and to maximize its impact on renewable energy portfolios. Numerous studies have shown that soil moisture distribution and land surface vegetative processes profoundly influence atmospheric boundary layer development and weather processes on local and regional scales. Using the PF.WRF model, a fully-coupled hydrologic and atmospheric model employing the ParFlow hydrologic model with the Weather Research and Forecasting model coupled via mass and energy fluxes across the land surface, we have explored the connections between the land surface and the atmosphere in terms of land surface energy flux partitioning and coupled variable fields including hydraulic conductivity, soil moisture and wind speed, and demonstrated that reductions in uncertainty in these coupled fields propagate through the hydrologic and atmospheric system. We have adapted the Data Assimilation Research Testbed (DART), an implementation of the robust Ensemble Kalman Filter data assimilation algorithm, to expand our capability to nudge forecasts produced with the PF.WRF model using observational data. Using a semi-idealized simulation domain, we examine the effects of assimilating observations of variables such as wind speed and temperature collected in the atmosphere, and land surface and subsurface observations such as soil moisture on the quality of forecast outputs. The sensitivities we find in this study will enable further studies to optimize observation collection to maximize the utility of the PF.WRF-DART forecasting system.

Towards improved capability and confidence in coupled atmospheric and wildland fire modeling

NASA Astrophysics Data System (ADS)

Sauer, Jeremy A.

This dissertation work is aimed at improving the capability and confidence in a modernized and improved version of Los Alamos National Laboratory's coupled atmospheric and wild- land fire dynamics model, Higrad-Firetec. Higrad is the hydrodynamics component of this large eddy simulation model that solves the three dimensional, fully compressible Navier-Stokes equations, incorporating a dynamic eddy viscosity formulation through a two-scale turbulence closure scheme. Firetec is the vegetation, drag forcing, and combustion physics portion that is integrated with Higrad. The modern version of Higrad-Firetec incorporates multiple numerical methodologies and high performance computing aspects which combine to yield a unique tool capable of augmenting theoretical and observational investigations in order to better understand the multi-scale, multi-phase, and multi-physics, phenomena involved in coupled atmospheric and environmental dynamics. More specifically, the current work includes extended functionality and validation efforts targeting component processes in coupled atmospheric and wildland fire scenarios. Since observational data of sufficient quality and resolution to validate the fully coupled atmosphere-wildfire scenario simply does not exist, we instead seek to validate components of the full prohibitively convoluted process. This manuscript provides first, an introduction and background into the application space of Higrad-Firetec. Second we document the model formulation, solution procedure, and a simple scalar transport verification exercise. Third, we perform a validate model results against observational data for time averaged flow field metrics in and above four idealized forest canopies. Fourth, we carry out a validation effort for the non-buoyant jet in a crossflow scenario (to which an analogy can be made for atmosphere-wildfire interactions) comparing model results to laboratory data of both steady-in-time and unsteady-in-time metrics. Finally, an extension of model multi-phase physics is implemented, allowing for the representation of multiple collocated fuels as separately evolving constituents leading to differences resulting rate of spread and total burned area. In combination these efforts demonstrate improved capability, increased validation of component functionality, and unique applicability the Higrad-Firetec modeling framework. As a result this work provides a substantially more robust foundation for future new, more widely acceptable investigations into the complexities of coupled atmospheric and wildland fire behavior.

Development and application of a regional-scale atmospheric mercury model based on WRF/Chem: a Mediterranean area investigation.

PubMed

Gencarelli, Christian Natale; De Simone, Francesco; Hedgecock, Ian Michael; Sprovieri, Francesca; Pirrone, Nicola

2014-03-01

The emission, transport, deposition and eventual fate of mercury (Hg) in the Mediterranean area has been studied using a modified version of the Weather Research and Forecasting model coupled with Chemistry (WRF/Chem). This model version has been developed specifically with the aim to simulate the atmospheric processes determining atmospheric Hg emissions, concentrations and deposition online at high spatial resolution. For this purpose, the gas phase chemistry of Hg and a parametrised representation of atmospheric Hg aqueous chemistry have been added to the regional acid deposition model version 2 chemical mechanism in WRF/Chem. Anthropogenic mercury emissions from the Arctic Monitoring and Assessment Programme included in the emissions preprocessor, mercury evasion from the sea surface and Hg released from biomass burning have also been included. Dry and wet deposition processes for Hg have been implemented. The model has been tested for the whole of 2009 using measurements of total gaseous mercury from the European Monitoring and Evaluation Programme monitoring network. Speciated measurement data of atmospheric elemental Hg, gaseous oxidised Hg and Hg associated with particulate matter, from a Mediterranean oceanographic campaign (June 2009), has permitted the model's ability to simulate the atmospheric redox chemistry of Hg to be assessed. The model results highlight the importance of both the boundary conditions employed and the accuracy of the mercury speciation in the emission database. The model has permitted the reevaluation of the deposition to, and the emission from, the Mediterranean Sea. In light of the well-known high concentrations of methylmercury in a number of Mediterranean fish species, this information is important in establishing the mass balance of Hg for the Mediterranean Sea. The model results support the idea that the Mediterranean Sea is a net source of Hg to the atmosphere and suggest that the net flux is ≈30 Mg year(-1) of elemental Hg.

Assessing the atmospheric and climatic effects of basaltic fissure eruptions. A case study Nornahraun, North Iceland, 2014-2015.

NASA Astrophysics Data System (ADS)

Gallagher, Catherine; Burton, Kevin; Thordarson, Thorvaldur; Vye-Brown, Charlotte; Brown, Richard

2015-04-01

A volcanic eruption's ability to release sulphur gases into the atmosphere is one of the critical factors in assessing their climatic and environmental effects, because it is directly linked to the potential H2SO4 aerosol burden produced [1]. Basaltic fissure eruptions loft large amounts of sulphur into the atmosphere because of the efficient degassing of volatiles and halogens from the magma at the vent [2-4] coupled with the high sulphur yield of basaltic magma. The common nature of this style of eruption and its products, regardless of magnitude, means that our understanding of the exact processes which influence atmospheric chemistry and environmental impact is very important. The Nornahraun fissure eruption in North Iceland that began on the 31st August 2014, has quickly become one of the best documented eruptions of its kind, through systematic monitoring and sampling by the Institute of Earth Sciences eruption team and The Icelandic Meteorological Office. As a result it is an excellent modern analogue for historic or ancient basaltic fissure eruptions, for which the amount of degassing can only be estimated through petrological and geochemical methods. It also serves as a timely testing platform for novel geochemical proxies. This study uses the exceptional sensitivity of the 187Os-187Re radiogenic system to the presence of crustal material [5], and highly siderophile stable isotopes Cu, Zn and S to indicate the chemistry and degassing of the melt carrying S to the surface. The geochemical isotopic proxies will be tested using established petrological methods and gas emission data. This study concentrates on determining the following key parameters: (1) The source of volatiles in the magma indicated though the pressure dependence of S solubility. (2) The mechanism of aerosol and gas release into the atmosphere is dictated both by the chemistry of the melt that controls the S species (H2S, SO2 or FeS2) present [6], and by the mechanism of transfer. (3) The amount of volatiles released during a basaltic fissure eruption both at the vent (>70%) as well as during lava transport [2-4]. This uses the petrological method of Devine et al (1984) and a two-stage degassing model [3] to establish the total S budget. (4) The duration of atmospheric loading of volatiles in an eruption, which affects the residence time of these gases and aerosols. The Nornahraun event provides the opportunity to verify the gas species and aerosols present in the atmosphere. By utilising the very well documented Nornahraun eruption, better constraints can be obtained on the atmospheric effects of well-known historical eruptions such as Laki 1783-84. Scaling up of such models to large flood basalt eruptions may shed light on their climatic effects and postulated association with major mass extinctions. [1] Thordarson, T. et al. Geol. Soc. London. Spec. Publ. 213 (2003), 103-121. [2] Guilbaud, M.-N. et al. Journal of Petrology 48.(2007), 1265-1294. [3] Thordarson, T. et al. Bulletin of Volcanology 58.(1996), 205-225. [4] Metrich, N. et al. Contrib Mineraology Petrol 107.(1991), 435-447. [5]Gannoun, A. et al. Science 303.(2004),70-72. [6] Burgisser, A., Scaillet, B. Nature 445.(2007), 194-197.

Initialization and Predictability of a Coupled ENSO Forecast Model

NASA Technical Reports Server (NTRS)

Chen, Dake; Zebiak, Stephen E.; Cane, Mark A.; Busalacchi, Antonio J.

1997-01-01

The skill of a coupled ocean-atmosphere model in predicting ENSO has recently been improved using a new initialization procedure in which initial conditions are obtained from the coupled model, nudged toward observations of wind stress. The previous procedure involved direct insertion of wind stress observations, ignoring model feedback from ocean to atmosphere. The success of the new scheme is attributed to its explicit consideration of ocean-atmosphere coupling and the associated reduction of "initialization shock" and random noise. The so-called spring predictability barrier is eliminated, suggesting that such a barrier is not intrinsic to the real climate system. Initial attempts to generalize the nudging procedure to include SST were not successful; possible explanations are offered. In all experiments forecast skill is found to be much higher for the 1980s than for the 1970s and 1990s, suggesting decadal variations in predictability.

Application of a Mesoscale Atmospheric Coupled Fire Model BRAMS-FIRE to Alentejo Woodland Fire and Comparison of Performance with the Fire Model WRF-Sfire.

NASA Astrophysics Data System (ADS)

Freitas, S. R.; Menezes, I. C.; Stockler, R.; Mello, R.; Ribeiro, N. A.; Corte-Real, J. A. M.; Surový, P.

2014-12-01

Models of fuel with the identification of vegetation patterns of Montado ecosystem in Portugal was incorporated in the mesoscale Brazilian Atmospheric Modeling System (BRAMS) and coupled with a spread woodland fire model. The BRAMS-FIRE is a new system developed by the "Centro de Previsão de Tempo e Estudos Climáticos" (CPTEC/INPE, Brazil) and the "Instituto de Ciências Agrárias e Ambientais Mediterrâneas" (ICAAM, Portugal). The fire model used in this effort was originally, developed by Mandel et al. (2013) and further incorporated in the Weather Research and Forecast model (WRF). Two grids of high spatial resolution were configured with surface input data and fuel models integrated for simulations using both models BRAMS-FIRE and WRF-SFIRE. One grid was placed in the plain land near Beja and the other one in the hills of Ossa to evaluate different types of fire propagation and calibrate BRAMS-FIRE. The objective is simulating the effects of atmospheric circulation in local scale, namely the movements of the heat front and energy release associated to it, obtained by this two models in an episode of woodland fire which took place in Alentejo area in the last decade, for application to planning and evaluations of agro woodland fire risks. We aim to model the behavior of forest fires through a set of equations whose solutions provide quantitative values of one or more variables related to the propagation of fire, described by semi-empirical expressions that are complemented by experimental data allow to obtain the main variables related advancing the perimeter of the fire, as the propagation speed, the intensity of the fire front and fuel consumption and its interaction with atmospheric dynamic system. References Mandel, J., J. D. Beezley, G. Kelman, A. K. Kochanski, V. Y. Kondratenko, B. H. Lynn, and M. Vejmelka, 2013. New features in WRF-SFIRE and the wildfire forecasting and danger system in Israel. Natural Hazards and Earth System Sciences, submitted, Numerical Wildfires, Cargèse, France, May 13-18, 2013.

Application of a mesoscale atmospheric coupled fire model BRAMS-SFIRE to Alentejo wildland fire and comparison of performance with the fire model WRF-SFIRE

NASA Astrophysics Data System (ADS)

Menezes, Isilda; Freitas, Saulo; Stockler, Rafael; Mello, Rafael; Ribeiro, Nuno; Corte-Real, João; Surový, Peter

2015-04-01

Models of fuel with the identification of vegetation patterns of Montado ecosystem in Portugal was incorporated in the mesoscale Brazilian Atmospheric Modeling System (BRAMS) and coupled with a spread wildland fire model. The BRAMS-FIRE is a new system developed by the Centro de Previsão de Tempo e Estudos Climáticos (CPTEC/INPE, Brazil) and the Instituto de Ciências Agrárias e Ambientais Mediterrâneas (ICAAM, Portugal). The fire model used in this effort was originally, developed by Mandel et al. (2013) and further incorporated in the Weather Research and Forecast model (WRF). Two grids of high spatial resolution were configured with surface input data and fuel models integrated for simulations using both models BRAMS-SFIRE and WRF-SFIRE. One grid was placed in the plain land and the other one in the hills to evaluate different types of fire propagation and calibrate BRAMS-SFIRE. The objective is simulating the effects of atmospheric circulation in local scale, namely the movements of the heat front and energy release associated to it, obtained by this two models in an episode of wildland fire which took place in Alentejo area in the last decade, for application to planning and evaluations of agro wildland fire risks. We aim to model the behavior of forest fires through a set of equations whose solutions provide quantitative values of one or more variables related to the propagation of fire, described by semi-empirical expressions that are complemented by experimental data allow to obtain the main variables related advancing the perimeter of the fire, as the propagation speed, the intensity of the fire front and fuel consumption and its interaction with atmospheric dynamic system References Mandel, J., J. D. Beezley, G. Kelman, A. K. Kochanski, V. Y. Kondratenko, B. H. Lynn, and M. Vejmelka, 2013. New features in WRF-SFIRE and the wildfire forecasting and danger system in Israel. Natural Hazards and Earth System Sciences, submitted, Numerical Wildfires, Cargèse, France, May 13-18, 2013.

Seasonal simulations using a coupled ocean-atmosphere model with data assimilation

NASA Astrophysics Data System (ADS)

Larow, Timothy Edward

1997-10-01

A coupled ocean-atmosphere initialization scheme using Newtonian relaxation has been developed for the Florida State University coupled ocean-atmosphere global general circulation model. The coupled model is used for seasonal predictions of the boreal summers of 1987 and 1988. The atmosphere model is a modified version of the Florida State University global spectral model, resolution triangular truncation 42 waves. The ocean general circulation model consists of a slightly modified version developed by Latif (1987). Coupling is synchronous with exchange of information every two model hours. Using daily analysis from ECMWF and observed monthly mean SSTs from NCEP, two - one year, time dependent, Newtonian relaxation were conducted using the coupled model prior to the seasonal forecasts. Relaxation was selectively applied to the atmospheric vorticity, divergence, temperature, and dew point depression equations, and to the ocean's surface temperature equation. The ocean's initial conditions are from a six year ocean-only simulation which used observed wind stresses and a relaxation towards observed SSTs for forcings. Coupled initialization was conducted from 1 June 1986 to 1 June 1987 for the 1987 boreal forecast and from 1 June 1987 to 1 June 1988 for the 1988 boreal forecast. Examination of annual means of net heat flux, freshwater flux and wind stress obtained by from the initialization show close agreement with Oberhuber (1988) climatology and the Florida State University pseudo wind stress analysis. Sensitivity of the initialization/assimilation scheme was tested by conducting two - ten member ensemble integrations. Each member was integrated for 90 days (June-August) of the respective year. Initial conditions for the ensembles consisted of the same ocean state as used by the initialize forecasts, while the atmospheric initial conditions were from ECMWF analysis centered on 1 June of the respective year. Root mean square error and anomaly correlations between observed and forecasted SSTs in the Nino 3 and Nino 4 regions show greater skill between the initialized forecasts than the ensemble forecasts. It is hypothesized that differences in the specific humidity within the planetary boundary layer are responsible for the large SST errors noted with the ensembles.

Modeling Atmospheric CO2 Processes to Constrain the Missing Sink

NASA Technical Reports Server (NTRS)

Kawa, S. R.; Denning, A. S.; Erickson, D. J.; Collatz, J. C.; Pawson, S.

2005-01-01

We report on a NASA supported modeling effort to reduce uncertainty in carbon cycle processes that create the so-called missing sink of atmospheric CO2. Our overall objective is to improve characterization of CO2 source/sink processes globally with improved formulations for atmospheric transport, terrestrial uptake and release, biomass and fossil fuel burning, and observational data analysis. The motivation for this study follows from the perspective that progress in determining CO2 sources and sinks beyond the current state of the art will rely on utilization of more extensive and intensive CO2 and related observations including those from satellite remote sensing. The major components of this effort are: 1) Continued development of the chemistry and transport model using analyzed meteorological fields from the Goddard Global Modeling and Assimilation Office, with comparison to real time data in both forward and inverse modes; 2) An advanced biosphere model, constrained by remote sensing data, coupled to the global transport model to produce distributions of CO2 fluxes and concentrations that are consistent with actual meteorological variability; 3) Improved remote sensing estimates for biomass burning emission fluxes to better characterize interannual variability in the atmospheric CO2 budget and to better constrain the land use change source; 4) Evaluating the impact of temporally resolved fossil fuel emission distributions on atmospheric CO2 gradients and variability. 5) Testing the impact of existing and planned remote sensing data sources (e.g., AIRS, MODIS, OCO) on inference of CO2 sources and sinks, and use the model to help establish measurement requirements for future remote sensing instruments. The results will help to prepare for the use of OCO and other satellite data in a multi-disciplinary carbon data assimilation system for analysis and prediction of carbon cycle changes and carbodclimate interactions.

Observed decrease in atmospheric mercury explained by global decline in anthropogenic emissions

PubMed Central

Zhang, Yanxu; Jacob, Daniel J.; Horowitz, Hannah M.; Chen, Long; Amos, Helen M.; Krabbenhoft, David P.; Slemr, Franz; St. Louis, Vincent L.; Sunderland, Elsie M.

2016-01-01

Observations of elemental mercury (Hg0) at sites in North America and Europe show large decreases (∼1–2% y−1) from 1990 to present. Observations in background northern hemisphere air, including Mauna Loa Observatory (Hawaii) and CARIBIC (Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container) aircraft flights, show weaker decreases (<1% y−1). These decreases are inconsistent with current global emission inventories indicating flat or increasing emissions over that period. However, the inventories have three major flaws: (i) they do not account for the decline in atmospheric release of Hg from commercial products; (ii) they are biased in their estimate of artisanal and small-scale gold mining emissions; and (iii) they do not properly account for the change in Hg0/HgII speciation of emissions from coal-fired utilities after implementation of emission controls targeted at SO2 and NOx. We construct an improved global emission inventory for the period 1990 to 2010 accounting for the above factors and find a 20% decrease in total Hg emissions and a 30% decrease in anthropogenic Hg0 emissions, with much larger decreases in North America and Europe offsetting the effect of increasing emissions in Asia. Implementation of our inventory in a global 3D atmospheric Hg simulation [GEOS-Chem (Goddard Earth Observing System-Chemistry)] coupled to land and ocean reservoirs reproduces the observed large-scale trends in atmospheric Hg0 concentrations and in HgII wet deposition. The large trends observed in North America and Europe reflect the phase-out of Hg from commercial products as well as the cobenefit from SO2 and NOx emission controls on coal-fired utilities. PMID:26729866

Observed decrease in atmospheric mercury explained by global decline in anthropogenic emissions.

PubMed

Zhang, Yanxu; Jacob, Daniel J; Horowitz, Hannah M; Chen, Long; Amos, Helen M; Krabbenhoft, David P; Slemr, Franz; St Louis, Vincent L; Sunderland, Elsie M

2016-01-19

Observations of elemental mercury (Hg(0)) at sites in North America and Europe show large decreases (∼ 1-2% y(-1)) from 1990 to present. Observations in background northern hemisphere air, including Mauna Loa Observatory (Hawaii) and CARIBIC (Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container) aircraft flights, show weaker decreases (<1% y(-1)). These decreases are inconsistent with current global emission inventories indicating flat or increasing emissions over that period. However, the inventories have three major flaws: (i) they do not account for the decline in atmospheric release of Hg from commercial products; (ii) they are biased in their estimate of artisanal and small-scale gold mining emissions; and (iii) they do not properly account for the change in Hg(0)/Hg(II) speciation of emissions from coal-fired utilities after implementation of emission controls targeted at SO2 and NOx. We construct an improved global emission inventory for the period 1990 to 2010 accounting for the above factors and find a 20% decrease in total Hg emissions and a 30% decrease in anthropogenic Hg(0) emissions, with much larger decreases in North America and Europe offsetting the effect of increasing emissions in Asia. Implementation of our inventory in a global 3D atmospheric Hg simulation [GEOS-Chem (Goddard Earth Observing System-Chemistry)] coupled to land and ocean reservoirs reproduces the observed large-scale trends in atmospheric Hg(0) concentrations and in Hg(II) wet deposition. The large trends observed in North America and Europe reflect the phase-out of Hg from commercial products as well as the cobenefit from SO2 and NOx emission controls on coal-fired utilities.

Radon observations as an integrated part of the multi parameter approach to study pre-earthquake processes

NASA Astrophysics Data System (ADS)

Ouzounov, Dimitar; Pulinets, Sergey; Lee, Lou; Giuliani, Guachino; Fu, Ching-Chou; Liu, Tiger; Hattori, Katsumi

2017-04-01

This work is part of international project to study the complex chain of interactions Lithosphere - Atmosphere -Ionosphere (LAI) in presence of ionization in atmosphere loaded by radon and other gases and is supported by International Space Science Institute (ISSI) in Bern and Beijing. We are presenting experimental measurements and theoretical estimates showing that radon measurements recorded before large earthquake are correlated with release of the heat flux in atmosphere during ionization of the atmospheric boundary layer .The recorded anomalous heat (observed by the remote sounding -infrared radiometers installed on satellites) are followed also by ionospheric anomalies (observed by GPS/TEC, ionosonde or satellite instruments). As ground proof we are using radon measurements installed and coordinated in four different seismic active regions California, Taiwan, Italy and Japan. Radon measurements are performed indirectly by means of gamma ray spectrometry of its radioactive progenies 214Pb and 214Bi (emitted at 351 keV and 609 keV, respectively) and also by Alfa detectors. We present data of five physical parameters- radon, seismicity, temperature of the atmosphere boundary layer, outgoing earth infrared radiation and GPS/TEC and their temporal and spatial variations several days before the onset of the following recent earthquakes: (1) 2016 M6.6 in California; (2) 2016 Amatrice-Norcia (Central Italy), (3) 2016 M6.4 of Feb 06 in Taiwan and (4) 2016 M7.0 of Nov 21 in Japan. Our preliminary results of simultaneous analysis of radon and space measurements in California, Italy, Taiwan and Japan suggests that pre-earthquake phase follows a general temporal-spatial evolution pattern in which radon plays a critical role in understanding the LAI coupling. This pattern could be reviled only with multi instruments observations and been seen and in other large earthquakes worldwide.

Evaluation of snowmelt simulation in the Weather Research and Forecasting model

NASA Astrophysics Data System (ADS)

Jin, Jiming; Wen, Lijuan

2012-05-01

The objective of this study is to better understand and improve snowmelt simulations in the advanced Weather Research and Forecasting (WRF) model by coupling it with the Community Land Model (CLM) Version 3.5. Both WRF and CLM are developed by the National Center for Atmospheric Research. The automated Snow Telemetry (SNOTEL) station data over the Columbia River Basin in the northwestern United States are used to evaluate snowmelt simulations generated with the coupled WRF-CLM model. These SNOTEL data include snow water equivalent (SWE), precipitation, and temperature. The simulations cover the period of March through June 2002 and focus mostly on the snowmelt season. Initial results show that when compared to observations, WRF-CLM significantly improves the simulations of SWE, which is underestimated when the release version of WRF is coupled with the Noah and Rapid Update Cycle (RUC) land surface schemes, in which snow physics is oversimplified. Further analysis shows that more realistic snow surface energy allocation in CLM is an important process that results in improved snowmelt simulations when compared to that in Noah and RUC. Additional simulations with WRF-CLM at different horizontal spatial resolutions indicate that accurate description of topography is also vital to SWE simulations. WRF-CLM at 10 km resolution produces the most realistic SWE simulations when compared to those produced with coarser spatial resolutions in which SWE is remarkably underestimated. The coupled WRF-CLM provides an important tool for research and forecasts in weather, climate, and water resources at regional scales.

Thermal stability of inorganic and organic compounds in atmospheric particulate matter

NASA Astrophysics Data System (ADS)

Perrino, Cinzia; Marconi, Elisabetta; Tofful, Luca; Farao, Carmela; Materazzi, Stefano; Canepari, Silvia

2012-07-01

The thermal behaviour of atmospheric particulate matter (PM) has been investigated by using different analytical approaches to explore the added value offered by these technique in environmental studies. The thermogravimetric analysis (TGA), carried out on both certified material and real PM samples, has shown that several mass losses can be detected starting from 80 °C up to above 500 °C, when pyrolysis occur. Thermo-optical analysis of PM and ion chromatographic analysis of the residual have shown that the mass losses in the temperature range 80-180 °C are not justified by the release of either organic or inorganic compounds; it can be thus attributed to the release of weakly and strongly bound water. Release of water has also been evidenced in the temperature range 225-275 °C. The release of ammonium chloride and nitrate has been detected only above 80 °C. This indicates that the release of nitric acid, hydrochloric acid and ammonia, which is observed downstream of the filters during the sampling of atmospheric PM at ambient temperature, cannot be reproduced off-line, after the end of the sampling. We successfully explored one of the possible explanations, that is the desorption of HNO3, HCl and NH3 adsorbed on collected particles. NH4NO3 and NH4Cl, which can be thermally released by the filter, exhibit a different thermal behaviour from NaNO3 and NaCl, which are thermally stable up to 370 °C. This different behaviour can be used to discriminate between natural and secondary sources of atmospheric inorganic salts, as the interconversion that is observed when heating mixtures of pure salts resulted to be not relevant when heating real PM samples.

Distribution of radionuclides between atmosphere and ash during combustion of contaminated vegetation.

PubMed

Zhou, Liufang Jenny; Rao, Raghu; Corcoran, Emily; Kelly, David

2016-12-01

A series of laboratory-scale combustion tests were conducted under well-controlled conditions to measure the release of 90 Sr and 137 Cs nuclides to the atmosphere (air) from combustion of vegetation and organic soil samples contaminated with radioactivity. These vegetation and soil samples were collected from a controlled contaminated forest area within the Canadian Nuclear Laboratories - Chalk River site. The combustion products including ash and smoke particulates, along with gaseous emissions, were collected and then analyzed for 137 Cs and 90 Sr concentrations by radiometric techniques. The experimental results reveal that the releases of 90 Sr to the atmosphere (air) from combustion of vegetation are very low with most of the 90 Sr activity remaining in ash residues, even at a temperature of 800 °C. The detailed combustion experiments with surface litter and twigs, alder twigs, alder leaves, and organic soil indicate that 0.5 ± 0.1%, 0.3 ± 0.1%, 0.9 ± 0.1%, and 0.3 ± 0.1% of 90 Sr is released to the atmosphere (air), respectively. On the other hand, the releases of 137 Cs are found to be highly dependent on the combustion temperature as well as the nature of vegetation. The releases of 137 Cs obtained at 800 °C are 45 ± 7%, 77 ± 9%, 92 ± 5%, and 2.4 ± 0.5% for surface litter and twigs, alder twigs, alder leaves, and organic soil, respectively. The mechanism associated with the high release of 137 Cs at a high temperature of 800 °C was explored. Crown Copyright © 2016. Published by Elsevier Ltd. All rights reserved.

Assessment of plutonium in the Savannah River Site environment. Revision 1

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carlton, W.H.; Evans, A.G.; Geary, L.A.

1992-12-31

Plutonium in the Savannah River Site Environment is published as a part of the Radiological Assessment Program (RAP). It is the fifth in a series of eight documents on individual radioisotopes released to the environment as a result of Savannah River Site (SRS) operations. These are living documents, each to be revised and updated on a two-year schedule. This document describes the sources of plutonium in the environment, its release from SRS, environmental transport and ecological concentration of plutonium, and the radiological impact of SRS releases to the environment. Plutonium exists in the environment as a result of above-ground nuclearmore » weapons tests, the Chernobyl accident, the destruction of satellite SNAP 9-A, plane crashes involving nuclear weapons, and small releases from reactors and reprocessing plants. Plutonium has been produced at SRS during the operation of five production reactors and released in small quantities during the processing of fuel and targets in chemical separations facilities. Approximately 0.6 Ci of plutonium was released into streams and about 12 Ci was released to seepage basins, where it was tightly bound by clay in the soil. A smaller quantity, about 3.8 Ci, was released to the atmosphere. Virtually all releases have occurred in F- and H-Area separation facilities. Plutonium concentration and transport mechanisms for the atmosphere, surface water, and ground water releases have been extensively studied by Savannah River Technology Center (SRTC) and ecological mechanisms have been studied by Savannah River Ecology Laboratory (SREL). The overall radiological impact of SRS releases to the offsite maximum individual can be characterized by a total dose of 15 mrem (atmospheric) and 0.18 mrem (liquid), compared with the dose of 12,960 mrem from non-SRS sources during the same period of time (1954--1989). Plutonium releases from SRS facilities have resulted in a negligible impact to the environment and the population it supports.« less

Comparison of MERRA-2 and ECCO-v4 ocean surface heat fluxes: Consequences of different forcing feedbacks on ocean circulation and implications for climate data assimilation.

NASA Astrophysics Data System (ADS)

Strobach, E.; Molod, A.; Menemenlis, D.; Forget, G.; Hill, C. N.; Campin, J. M.; Heimbach, P.

2017-12-01

Forcing ocean models with reanalysis data is a common practice in ocean modeling. As part of this practice, prescribed atmospheric state variables and interactive ocean SST are used to calculate fluxes between the ocean and the atmosphere. When forcing an ocean model with reanalysis fields, errors in the reanalysis data, errors in the ocean model and errors in the forcing formulation will generate a different solution compared to other ocean reanalysis solutions (which also have their own errors). As a first step towards a consistent coupled ocean-atmosphere reanalysis, we compare surface heat fluxes from a state-of-the-art atmospheric reanalysis, the Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), to heat fluxes from a state-of-the-art oceanic reanalysis, the Estimating the Circulation and Climate of the Ocean Version 4, Release 2 (ECCO-v4). Then, we investigate the errors associated with the MITgcm ocean model in its ECCO-v4 ocean reanalysis configuration (1992-2011) when it is forced with MERRA-2 atmospheric reanalysis fields instead of with the ECCO-v4 adjoint optimized ERA-interim state variables. This is done by forcing ECCO-v4 ocean with and without feedbacks from MERRA-2 related to turbulent fluxes of heat and moisture and the outgoing long wave radiation. In addition, we introduce an intermediate forcing method that includes only the feedback from the interactive outgoing long wave radiation. The resulting ocean circulation is compared with ECCO-v4 reanalysis and in-situ observations. We show that, without feedbacks, imbalances in the energy and the hydrological cycles of MERRA-2 (which are directly related to the fact it was created without interactive ocean) result in considerable SST drifts and a large reduction in sea level. The bulk formulae and interactive outgoing long wave radiation, although providing air-sea feedbacks and reducing model-data misfit, strongly relax the ocean to observed SST and may result in unwanted features such as large change in the water budget. These features have implications in on desired forcing recipe to be used. The results strongly and unambiguously argue for next generation data assimilation climate studies to involve fully coupled systems.

Middle atmosphere electrodynamics: Report of the workshop on the Role of the Electrodynamics of the Middle Atmosphere on Solar Terrestrial Coupling

NASA Technical Reports Server (NTRS)

Maynard, N. C. (Editor)

1979-01-01

Significant deficiencies exist in the present understanding of the basic physical processes taking place within the middle atmosphere (the region between the tropopause and the mesopause), and in the knowledge of the variability of many of the primary parameters that regulate Middle Atmosphere Electrodynamics (MAE). Knowledge of the electrical properties, i.e., electric fields, plasma characteristics, conductivity and currents, and the physical processes that govern them is of fundamental importance to the physics of the region. Middle atmosphere electrodynamics may play a critical role in the electrodynamical aspects of solar-terrestrial relations. As a first step, the Workshop on the Role of the Electrodynamics of the Middle Atmosphere on Solar-Terrestrial Coupling was held to review the present status and define recommendations for future MAE research.

A quasi-static model of global atmospheric electricity. II - Electrical coupling between the upper and lower atmosphere

NASA Technical Reports Server (NTRS)

Roble, R. G.; Hays, P. B.

1979-01-01

The paper presents a model of global atmospheric electricity used to examine the effect of upper atmospheric generators on the global electrical circuit. The model represents thunderstorms as dipole current generators randomly distributed in areas of known thunderstorm frequency; the electrical conductivity in the model increases with altitude, and electrical effects are coupled with a passive magnetosphere along geomagnetic field lines. The large horizontal-scale potential differences at ionospheric heights map downward into the lower atmosphere where the perturbations in the ground electric field are superimposed on the diurnal variation. Finally, changes in the upper atmospheric conductivity due to solar flares, polar cap absorptions, and Forbush decreases are shown to alter the downward mapping of the high-latitude potential pattern and the global distribution of fields and currents.

Modeling coupled interactions of carbon, water, and ozone exchange between terrestrial ecosystems and the atmosphere

Treesearch

Ned Nikolova; Karl F. Zeller

2003-01-01

A new biophysical model (FORFLUX) is presented to study the simultaneous exchange of ozone, carbon dioxide, and water vapor between terrestrial ecosystems and the atmosphere. The model mechanistically couples all major processes controlling ecosystem flows trace gases and water implementing recent concepts in plant eco-physiology, micrometeorology, and soil hydrology....

WET EFFLUENT PARALLEL PLATE DIFFUSION DENUDER COUPLED CAPILLARY ION CHROMATOGRAPH FOR THE DETERMINATION OF ATMOSPHERIC TRACE GASES. (R825344)

EPA Science Inventory

We describe an inexpensive, compact parallel plate diffusion denuder coupled capillary IC system for the determination of soluble ionogenic atmospheric trace gases. The active sampling area (0.6×10 cm) of the denuder is formed in a novel manner by thermally bonding silica ge...

A case study of convectively generated gravity waves coupling of the lower atmosphere and mesosphere-lower thermosphere (MLT) over the tropical region: An observational evidence

NASA Astrophysics Data System (ADS)

Eswaraiah, S.; Venkata Chalapathi, G.; Niranjan Kumar, K.; Venkat Ratnam, M.; Kim, Yong Ha; Vishnu Prasanth, P.; Lee, Jaewook; Rao, S. V. B.

2018-04-01

We have utilized the Gadanki MST Radar and Rayleigh LIDAR to understand the vertical coupling between the lower atmosphere and mesosphere through the short-period gravity waves (GWs). The short-period GWs (20 min-2 h) are noticed both in the troposphere and in the mesosphere during the deep convection. During the convection, the large vertical velocities (>5 m/s) and significant variations in the momentum flux (∼3 m2/s2) are noticed in the troposphere and higher fluxes (∼45 m2/s2) are evidenced in the mesosphere. The observations suggest the vertical coupling between the lower and middle atmosphere during convection.

Modeling the volcanic signal in the atmospheric CO2 record

NASA Astrophysics Data System (ADS)

Jones, Chris D.; Cox, Peter M.

2001-06-01

There is significant interannual variability in the atmospheric concentration of carbon dioxide even when the effect of anthropogenic sources has been accounted for. It has been shown that this variability is correlated with the El Nino Southern Oscillation (ENSO) cycle [Bacastow, 1976; Keeling et al., 1995]. However, there are periods during the atmospheric CO2 record when this correlation does not hold and CO2 levels are much lower than can be explained by the correlation with ENSO. These periods coincide with major volcanic eruptions. It has been well documented that a major eruption has a cooling effect on the surface and lower troposphere [McCormick, 1992; Hansen, et al., 1996]. Here we show that it is likely that this cooling has a significant and measurable effect on the carbon cycle. We use a coupled general circulation climate-carbon cycle model to study the mechanisms involved. The model simulates the observed temperature and CO2 response of the climate to the 1991 eruption of Mount Pinatubo. The surface cooling due to the eruption leads to reduced soil and plant respiration globally and increased gross primary productivity in the tropics. The result is significant uptake of carbon (1-2 GtC yr-1) by the terrestrial biosphere for several years after the eruption. There is no significant variation in uptake or release of carbon by the oceans.

Theoretical Thermodynamics of Mixtures at High Pressures

NASA Technical Reports Server (NTRS)

Hubbard, W. B.

1985-01-01

The development of an understanding of the chemistry of mixtures of metallic hydrogen and abundant, higher-z material such as oxygen, carbon, etc., is important for understanding of fundamental processes of energy release, differentiation, and development of atmospheric abundances in the Jovian planets. It provides a significant theoretical base for the interpretation of atmospheric elemental abundances to be provided by atmospheric entry probes in coming years. Significant differences are found when non-perturbative approaches such as Thomas-Fermi-Dirac (TFD) theory are used. Mapping of the phase diagrams of such binary mixtures in the pressure range from approx. 10 Mbar to approx. 1000 Mbar, using results from three-dimensional TFD calculations is undertaken. Derivation of a general and flexible thermodynamic model for such binary mixtures in the relevant pressure range was facilitated by the following breakthrough: there exists an accurate nd fairly simple thermodynamic representation of a liquid two-component plasma (TCP) in which the Helmholtz free energy is represented as a suitable linear combination of terms dependent only on density and terms which depend only on the ion coupling parameter. It is found that the crystal energies of mixtures of H-He, H-C, and H-O can be satisfactorily reproduced by the same type of model, except that an effective, density-dependent ionic charge must be used in place of the actual total ionic charge.

Refining multi-model projections of temperature extremes by evaluation against land-atmosphere coupling diagnostics

NASA Astrophysics Data System (ADS)

Sippel, Sebastian; Zscheischler, Jakob; Mahecha, Miguel D.; Orth, Rene; Reichstein, Markus; Vogel, Martha; Seneviratne, Sonia I.

2017-05-01

The Earth's land surface and the atmosphere are strongly interlinked through the exchange of energy and matter. This coupled behaviour causes various land-atmosphere feedbacks, and an insufficient understanding of these feedbacks contributes to uncertain global climate model projections. For example, a crucial role of the land surface in exacerbating summer heat waves in midlatitude regions has been identified empirically for high-impact heat waves, but individual climate models differ widely in their respective representation of land-atmosphere coupling. Here, we compile an ensemble of 54 combinations of observations-based temperature (T) and evapotranspiration (ET) benchmarking datasets and investigate coincidences of T anomalies with ET anomalies as a proxy for land-atmosphere interactions during periods of anomalously warm temperatures. First, we demonstrate that a large fraction of state-of-the-art climate models from the Coupled Model Intercomparison Project (CMIP5) archive produces systematically too frequent coincidences of high T anomalies with negative ET anomalies in midlatitude regions during the warm season and in several tropical regions year-round. These coincidences (high T, low ET) are closely related to the representation of temperature variability and extremes across the multi-model ensemble. Second, we derive a land-coupling constraint based on the spread of the T-ET datasets and consequently retain only a subset of CMIP5 models that produce a land-coupling behaviour that is compatible with these benchmark estimates. The constrained multi-model simulations exhibit more realistic temperature extremes of reduced magnitude in present climate in regions where models show substantial spread in T-ET coupling, i.e. biases in the model ensemble are consistently reduced. Also the multi-model simulations for the coming decades display decreased absolute temperature extremes in the constrained ensemble. On the other hand, the differences between projected and present-day climate extremes are affected to a lesser extent by the applied constraint, i.e. projected changes are reduced locally by around 0.5 to 1 °C - but this remains a local effect in regions that are highly sensitive to land-atmosphere coupling. In summary, our approach offers a physically consistent, diagnostic-based avenue to evaluate multi-model ensembles and subsequently reduce model biases in simulated and projected extreme temperatures.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cochran, C.B.

This patent describes a double nut setting tool and liner hanger assembly. It comprises a tool which is releasably coupled to the liner hanger by a nut means threadedly connected to the liner hanger: upon reaching a desired setting location, hanging the liner hanger in the well to support the weight of the liner and to permit rotation of the liner: manipulating the string of pipe to simultaneously rotate the nut means to a released condition relative to the liner hanger while rotating a lock nut in a clutch housing into a locking position in the clutch housing to engagemore » the clutch housing with the liner; and applying weight to the string of pipe to engage the clutch housing with the liner when the coupling nut is released and the lock nut is in a locking position so that the liner can be rotated by rotation of the string of pipe after the coupling nut is released.« less

Ice core measurements of 14CH4 show no evidence of methane release to atmosphere from methane hydrates during a large warming event 11,600 years ago

NASA Astrophysics Data System (ADS)

Petrenko, V. V.; Severinghaus, J. P.; Smith, A.; Riedel, K.; Brook, E.; Schaefer, H.; Baggenstos, D.; Harth, C. M.; Hua, Q.; Buizert, C.; Schilt, A.; Fain, X.; Mitchell, L.; Bauska, T. K.; Orsi, A. J.; Weiss, R. F.

2016-12-01

Marine methane hydrate destabilization has been proposed as a potentially large source of methane to the atmosphere in response to both past and future warming. We present new measurements of 14C of paleoatmospheric methane (CH4) over the Younger Dryas - Preboreal (YD - PB) abrupt warming event (≈11,600 years ago) from ancient ice outcropping at Taylor Glacier, Antarctica. The YD - PB abrupt warming was centered in the North Atlantic, occurred partway through the global warming of last deglaciation and was associated with a ≈ 50% increase in atmospheric CH4 concentrations. 14C can unambiguously identify CH4 emissions from "old carbon" sources, such as CH4 hydrates. All samples from before, during and after the abrupt warming and associated CH4 increase yielded 14CH4 values that are consistent with 14C of atmospheric CO2 at that time, indicating a purely contemporaneous methane source. Our results show that neither the abrupt regional warming nor the gradual global warming that preceded it resulted in detectable CH4 release to the atmosphere from CH4 hydrates during the YD - PB transition. Our results are thus consistent with the hypothesis that the vast majority of CH4 that is released from dissociating hydrates or other old-carbon seafloor CH4 sources is oxidized prior to reaching the atmosphere.

Interaction between protein kinase C and protein kinase A can modulate transmitter release at the rat neuromuscular synapse.

PubMed

Santafé, M M; Garcia, N; Lanuza, M A; Tomàs, M; Tomàs, J

2009-02-15

We used intracellular recording to investigate the functional interaction between protein kinase C (PKC) and protein kinase A (PKA) signal transduction cascades in the control of transmitter release in the neuromuscular synapses from adult rats. Our results indicate that: 1) PKA and PKC are independently involved in asynchronous release. 2) Evoked acetylcholine (ACh) release is enhanced with the PKA agonist Sp-8-BrcAMP and the PKC agonist phorbol ester (PMA). 3) PKA has a constitutive role in promoting a component of normal evoked transmitter release because, when the kinase is inhibited with H-89, the release diminishes. However, the PKC inhibitor calphostin C (CaC) does not affect ACh release. 4) PKA regulates neurotransmission without PKC involvement because, after PMA or CaC modulation of the PKC activity, coupling to the ACh release of PKA can normally be stimulated with Sp-8-BrcAMP or inhibited with H-89. 5) After PKA inhibition with H-89, PKC stimulation with PMA (or inhibition with CaC) does not lead to any change in evoked ACh release. However, in PKA-stimulated preparations with Sp-8-BrcAMP, PKC becomes tonically active, thus potentiating a component of release that can now be blocked with CaC. In normal conditions, therefore, PKA was able to modulate ACh release independently of PKC activity, whereas PKA stimulation caused the PKC coupling to evoked release. In contrast, PKA inhibition prevent PKC stimulation (with the phorbol ester) and coupling to ACh output. There was therefore some dependence of PKC on PKA activity in the fine control of the neuromuscular synaptic functionalism and ACh release.

Design and Impacts of Land-Biogenic-Atmosphere Coupling in the NASA-Unified WRF (NU-WRF) Modeling System

NASA Technical Reports Server (NTRS)

Tan, Qian; Santanello, Joseph A., Jr.; Zhou, Shujia; Tao, Zhining; Peters-Lidard, Christa d.; Chn, Mian

2011-01-01

Land-Atmosphere coupling is typically designed and implemented independently for physical (e.g. water and energy) and chemical (e.g. biogenic emissions and surface depositions)-based models and applications. Differences in scale, data requirements, and physics thus limit the ability of Earth System models to be fully coupled in a consistent manner. In order for the physical-chemical-biological coupling to be complete, treatment of the land in terms of surface classification, condition, fluxes, and emissions must be considered simultaneously and coherently across all components. In this study, we investigate a coupling strategy for the NASA-Unified Weather Research and Forecasting (NU-WRF) model that incorporates the traditionally disparate fluxes of water and energy through NASA's LIS (Land Information System) and biogenic emissions through BEIS (Biogenic Emissions Inventory System) and MEGAN (Model of Emissions of Gases and Aerosols from Nature) into the atmosphere. In doing so, inconsistencies across model inputs and parameter data are resolved such that the emissions from a particular plant species are consistent with the heat and moisture fluxes calculated for that land cover type. In turn, the response of the atmospheric turbulence and mixing in the planetary boundary layer (PBL) acts on the identical surface type, fluxes, and emissions for each. In addition, the coupling of dust emission within the NU-WRF system is performed in order to ensure consistency and to maximize the benefit of high-resolution land representation in LIS. The impacts of those self-consistent components on' the simulation of atmospheric aerosols are then evaluated through the WRF-Chem-GOCART (Goddard Chemistry Aerosol Radiation and Transport) model. Overall, this ambitious project highlights the current difficulties and future potential of fully coupled. components. in Earth System models, and underscores the importance of the iLEAPS community in supporting improved knowledge of processes and innovative approaches for models and observations.

Nicotinic Acid Adenine Dinucleotide Phosphate (NAADP) and Endolysosomal Two-pore Channels Modulate Membrane Excitability and Stimulus-Secretion Coupling in Mouse Pancreatic β Cells*

PubMed Central

Arredouani, Abdelilah; Ruas, Margarida; Collins, Stephan C.; Parkesh, Raman; Clough, Frederick; Pillinger, Toby; Coltart, George; Rietdorf, Katja; Royle, Andrew; Johnson, Paul; Braun, Matthias; Zhang, Quan; Sones, William; Shimomura, Kenju; Morgan, Anthony J.; Lewis, Alexander M.; Chuang, Kai-Ting; Tunn, Ruth; Gadea, Joaquin; Teboul, Lydia; Heister, Paula M.; Tynan, Patricia W.; Bellomo, Elisa A.; Rutter, Guy A.; Rorsman, Patrik; Churchill, Grant C.; Parrington, John; Galione, Antony

2015-01-01

Pancreatic β cells are electrically excitable and respond to elevated glucose concentrations with bursts of Ca2+ action potentials due to the activation of voltage-dependent Ca2+ channels (VDCCs), which leads to the exocytosis of insulin granules. We have examined the possible role of nicotinic acid adenine dinucleotide phosphate (NAADP)-mediated Ca2+ release from intracellular stores during stimulus-secretion coupling in primary mouse pancreatic β cells. NAADP-regulated Ca2+ release channels, likely two-pore channels (TPCs), have recently been shown to be a major mechanism for mobilizing Ca2+ from the endolysosomal system, resulting in localized Ca2+ signals. We show here that NAADP-mediated Ca2+ release from endolysosomal Ca2+ stores activates inward membrane currents and depolarizes the β cell to the threshold for VDCC activation and thereby contributes to glucose-evoked depolarization of the membrane potential during stimulus-response coupling. Selective pharmacological inhibition of NAADP-evoked Ca2+ release or genetic ablation of endolysosomal TPC1 or TPC2 channels attenuates glucose- and sulfonylurea-induced membrane currents, depolarization, cytoplasmic Ca2+ signals, and insulin secretion. Our findings implicate NAADP-evoked Ca2+ release from acidic Ca2+ storage organelles in stimulus-secretion coupling in β cells. PMID:26152717

The fate of cyanide in leach wastes at gold mines: an environmental perspective

USGS Publications Warehouse

Johnson, Craig A.

2015-01-01

Cyanide-containing and cyanide-related species are subject to attenuation mechanisms that lead to dispersal to the atmosphere, chemical transformation to other carbon and nitrogen species, or sequestration as cyanometallic precipitates or adsorbed species on mineral surfaces. Dispersal to the atmosphere and chemical transformation amount to permanent elimination of cyanide, whereas sequestration amounts to storage of cyanide in locations from which it can potentially be remobilized by infiltrating waters if conditions change. From an environmental perspective, the most significant cyanide releases from gold leach operations involve catastrophic spills of process solutions or leakage of effluent to the unsaturated or saturated zones. These release pathways are unfavorable for two important cyanide attenuation mechanisms that tend to occur naturally: dispersal of free cyanide to the atmosphere and sunlight-catalyzed dissociation of strong cyanometallic complexes, which produces free cyanide that can then disperse to the atmosphere. The widest margins of environmental safety will be achieved where mineral processing operations are designed so that time for offgassing, aeration, and sunlight exposure are maximized in the event that cyanide-bearing solutions are released inadvertently.

Atmospheric Renewable Energy Research, Volume 3: Solar-Power Microgrids and Atmospheric Influences

DTIC Science & Technology

2016-09-01

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Study of the effect of wind speed on evaporation from soil through integrated modeling of atmospheric boundary layer and shallow subsurface

NASA Astrophysics Data System (ADS)

Davarzani, Hossein; Smits, Kathleen; Tolene, Ryan; Illangasekare, Tissa

2013-04-01

The study of the interaction between the land and atmosphere is paramount to our understanding of many emerging problems to include climate change, the movement of green house gases such as possible leaking of sequestered CO2 and the accurate detection of buried objects such as landmines. Soil moisture distribution in the shallow subsurface becomes a critical factor in all these problems. The heat and mass flux in the form of soil evaporation across the land surface couples the atmospheric boundary layer to the shallow subsurface. The coupling between land and the atmosphere leads to highly dynamic interactions between the porous media properties, transport processes and boundary conditions, resulting in dynamic evaporative behavior. However, the coupling at the land-atmospheric interface is rarely considered in most current models and their validation for practical applications. This is due to the complexity of the problem in field scenarios and the scarcity of field or laboratory data capable of testing and refining coupled energy and mass transfer theories. In most efforts to compute evaporation from soil, only indirect coupling is provided to characterize the interaction between non-isothermal multiphase flows under realistic atmospheric conditions even though heat and mass flux are controlled by the coupled dynamics of the land and the atmospheric boundary layer. In earlier drying modeling concepts, imposing evaporation flux (kinetic of relative humidity) and temperature as surface boundary condition is often needed. With the goal of improving our understanding of the land/atmospheric coupling, we developed a model based on the coupling of Navier-Stokes free flow and Darcy flow in porous medium. The model consists of the coupled equations of mass conservation for the liquid phase (water) and gas phase (water vapor and air) in porous medium with gas phase (water vapor and air) in free flow domain under non-isothermal, non-equilibrium conditions. The boundary conditions at the porous medium-free flow medium interface include dynamical, thermal and solutal equilibriums, and using the Beavers-Joseph slip boundary condition. What is unique about this model is that the evaporation rate and soil surface temperature conditions come directly from the model output. In order to experimentally validate the numerical results, we developed and used a unique two dimensional wind tunnel placed above a soil tank equipped with a network of different sensors. A series of experiments under varying boundary conditions, using a test sand for which the hydraulic and thermal properties were well characterized, were performed. Precision data for soil moisture, soil and air temperature and relative humidity, and also wind velocity under well-controlled transient heat and wind boundary conditions was generated. Results from numerical simulations were compared with experimental data. Results demonstrate that the coupling concept can predict the different stages of the drying process in porous media with good accuracy. Increasing the wind speed increases the first stage evaporation rate and decreases the transition time at low velocity values; then, at high values of wind speed the evaporation rate becomes less dependent of flow in free fluid. In the opposite, the impact of the wind speed on the second stage evaporation (diffusion dominant stage) is not significant. The proposed theoretical model can be used to predict the evaporation process where a porous medium flow is coupled to a free flow for different practical applications.

Seismic generated infrasounds on Telluric Planets: Modeling and comparisons between Earth, Venus and Mars

NASA Astrophysics Data System (ADS)

Lognonne, P. H.; Rolland, L.; Karakostas, F. G.; Garcia, R.; Mimoun, D.; Banerdt, W. B.; Smrekar, S. E.

2015-12-01

Earth, Venus and Mars are all planets in which infrasounds can propagate and interact with the solid surface. This leads to infrasound generation for internal sources (e.g. quakes) and to seismic waves generations for atmospheric sources (e.g. meteor, impactor explosions, boundary layer turbulences). Both the atmospheric profile, surface density, atmospheric wind and viscous/attenuation processes are however greatly different, including major differences between Mars/Venus and Earth due to the CO2 molecular relaxation. We present modeling results and compare the seismic/acoustic coupling strength for Earth, Mars and Venus. This modeling is made through normal modes modelling for models integrating the interior, atmosphere, both with realistic attenuation (intrinsic Q for solid part, viscosity and molecular relaxation for the atmosphere). We complete these modeling, made for spherical structure, by integration of wind, assuming the later to be homogeneous at the scale of the infrasound wavelength. This allows us to compute either the Seismic normal modes (e.g. Rayleigh surface waves), or the acoustic or the atmospheric gravity modes. Comparisons are done, for either a seismic source or an atmospheric source, on the amplitude of expected signals as a function of distance and frequency. Effects of local time are integrated in the modeling. We illustrate the Rayleigh waves modelling by Earth data (for large quakes and volcanoes eruptions). For Venus, very large coupling can occur at resonance frequencies between the solid part and atmospheric part of the planet through infrasounds/Rayleigh waves coupling. If the atmosphere reduced the Q (quality coefficient) of Rayleigh waves in general, the atmosphere at these resonance soffers better propagation than Venus crust and increases their Q. For Mars, Rayleigh waves excitations by atmospheric burst is shown and discussed for the typical yield of impacts. The new data of the Nasa INSIGHT mission which carry both seismic and infrasound sensors will offer a unique confirmation in 2016-2017. We conclude with the seismic/infrasounds coupling on Venus which make the detection from space of seismic waves possible through the perturbation of the infrared airglow by infrassounds. Detection threshold as low as Magnitude 5.5 can be reached with existing technologies.

Diagnosing Air-Sea Interactions on Intraseasonal Timescales

NASA Astrophysics Data System (ADS)

DeMott, C. A.

2014-12-01

What is the role of ocean coupling in the Madden Julian Oscillation (MJO)? Consensus thinking holds that the essential physics of the MJO involve interactions between convection, atmospheric wave dynamics, and boundary layer and free troposphere moisture. However, many modeling studies demonstrate improved MJO simulation when an atmosphere-only general circulation model (AGCM) is coupled to an ocean model, so feedbacks from the ocean are probably not negligible. Assessing the importance and processes of these feedbacks is challenging for at least two reasons. First, observations of the MJO only sample the fully coupled ocean-atmosphere system; there is no "uncoupled" MJO in nature. Second, the practice of analyzing the MJO in uncoupled and coupled GCMs (CGCMs) involves using imperfect tools to study the problem. Although MJO simulation is improving in many models, shortcomings remain in both AGCMs and CGCMs, making it difficult to determine if changes brought about through coupling reflect critical air-sea interactions or are simply part of the collective idiosyncracies of a given model. For the atmosphere, ocean feedbacks from intraseasonal sea surface temperature (SST) variations are communicated through their effects on surface fluxes of heat and moisture. This presentation suggests a set of analysis tools for diagnosing the impact of an interactive ocean on surface latent and sensible heat fluxes, including their mean, variance, spectral characteristics, and phasing with respect to wind, SST, and MJO convection. The diagnostics are demonstrated with application to several CMIP5 models, and reveal a variety of responses to coupled ocean feedbacks.

Sensitivity of open-water ice growth and ice concentration evolution in a coupled atmosphere-ocean-sea ice model

NASA Astrophysics Data System (ADS)

Shi, Xiaoxu; Lohmann, Gerrit

2017-09-01

A coupled atmosphere-ocean-sea ice model is applied to investigate to what degree the area-thickness distribution of new ice formed in open water affects the ice and ocean properties. Two sensitivity experiments are performed which modify the horizontal-to-vertical aspect ratio of open-water ice growth. The resulting changes in the Arctic sea-ice concentration strongly affect the surface albedo, the ocean heat release to the atmosphere, and the sea-ice production. The changes are further amplified through a positive feedback mechanism among the Arctic sea ice, the Atlantic Meridional Overturning Circulation (AMOC), and the surface air temperature in the Arctic, as the Fram Strait sea ice import influences the freshwater budget in the North Atlantic Ocean. Anomalies in sea-ice transport lead to changes in sea surface properties of the North Atlantic and the strength of AMOC. For the Southern Ocean, the most pronounced change is a warming along the Antarctic Circumpolar Current (ACC), owing to the interhemispheric bipolar seasaw linked to AMOC weakening. Another insight of this study lies on the improvement of our climate model. The ocean component FESOM is a newly developed ocean-sea ice model with an unstructured mesh and multi-resolution. We find that the subpolar sea-ice boundary in the Northern Hemisphere can be improved by tuning the process of open-water ice growth, which strongly influences the sea ice concentration in the marginal ice zone, the North Atlantic circulation, salinity and Arctic sea ice volume. Since the distribution of new ice on open water relies on many uncertain parameters and the knowledge of the detailed processes is currently too crude, it is a challenge to implement the processes realistically into models. Based on our sensitivity experiments, we conclude a pronounced uncertainty related to open-water sea ice growth which could significantly affect the climate system sensitivity.

The role of spatial organization of Ca2+ release sites in the generation of arrhythmogenic diastolic Ca2+ release in myocytes from failing hearts

PubMed Central

Ho, Hsiang-Ting; Bonilla, Ingrid M.; Terentyeva, Radmila; Schober, Karsten E.; Terentyev, Dmitry; Carnes, Cynthia A.

2018-01-01

In heart failure (HF), dysregulated cardiac ryanodine receptors (RyR2) contribute to the generation of diastolic Ca2+ waves (DCWs), thereby predisposing adrenergically stressed failing hearts to life-threatening arrhythmias. However, the specific cellular, subcellular, and molecular defects that account for cardiac arrhythmia in HF remain to be elucidated. Patch-clamp techniques and confocal Ca2+ imaging were applied to study spatially defined Ca2+ handling in ventricular myocytes isolated from normal (control) and failing canine hearts. Based on their activation time upon electrical stimulation, Ca2+ release sites were categorized as coupled, located in close proximity to the sarcolemmal Ca2+ channels, and uncoupled, the Ca2+ channel-free non-junctional Ca2+ release units. In control myocytes, stimulation of β-adrenergic receptors with isoproterenol (Iso) resulted in a preferential increase in Ca2+ spark rate at uncoupled sites. This site-specific effect of Iso was eliminated by the phosphatase inhibitor okadaic acid, which caused similar facilitation of Ca2+ sparks at coupled and uncoupled sites. Iso-challenged HF myocytes exhibited increased predisposition to DCWs compared to control myocytes. In addition, the overall frequency of Ca2+ sparks was increased in HF cells due to preferential stimulation of coupled sites. Furthermore, coupled sites exhibited accelerated recovery from functional refractoriness in HF myocytes compared to control myocytes. Spatially resolved subcellular Ca2+ mapping revealed that DCWs predominantly originated from coupled sites. Inhibition of CaMK∏ suppressed DCWs and prevented preferential stimulation of coupled sites in Iso-challenged HF myocytes. These results suggest that CaMK∏-(and phosphatase)-dependent dysregulation of junctional Ca2+ release sites contributes to Ca2+-dependent arrhythmogenesis in HF. PMID:28612155

Global Coupled Carbon and Nitrogen Models: Successes, Failures and What next?

NASA Astrophysics Data System (ADS)

Holland, E. A.

2011-12-01

Over the last few years, there has been a great deal of progress in modeling coupled terrestrial global carbon and nitrogen cycles and their roles in Earth System models. The collection of recent models provides some surprising results and insights. A critical question for Earth system models is: How do the coupled C/N model results impact atmospheric carbon dioxide concentrations compared to carbon only models? Some coupled models predict increased atmospheric carbon dioxide concentrations, the result expected from nitrogen-limited photosynthesis uptake of carbon dioxide, while others predict little change or decreased carbon dioxide uptake with a coupled carbon and nitrogen cycle. With this range of impacts for climate critical atmospheric carbon dioxide concentrations, there is clearly a need for additional comparison of measurements and models. Randerson et al.'s CLAMP study provided important constraints and comparison for primarily for aboveground carbon uptake. However, nitrogen supply is largely determined decomposition and soil processes. I will present comparisons of NCAR's CESM results with soil and litter carbon and nitrogen fluxes and standing stocks. These belowground data sets of both carbon and nitrogen provide important benchmarks for coupled C/N models.

Study on power coupling of annular vortex beam propagating through a two-Cassegrain-telescope optical system in turbulent atmosphere.

PubMed

Wu, Huiyun; Sheng, Shen; Huang, Zhisong; Zhao, Siqing; Wang, Hua; Sun, Zhenhai; Xu, Xiegu

2013-02-25

As a new attractive application of the vortex beams, power coupling of annular vortex beam propagating through a two- Cassegrain-telescope optical system in turbulent atmosphere has been investigated. A typical model of annular vortex beam propagating through a two-Cassegrain-telescope optical system is established, the general analytical expression of vortex beams with limited apertures and the analytical formulas for the average intensity distribution at the receiver plane are derived. Under the H-V 5/7 turbulence model, the average intensity distribution at the receiver plane and power coupling efficiency of the optical system are numerically calculated, and the influences of the optical topological charge, the laser wavelength, the propagation path and the receiver apertures on the power coupling efficiency are analyzed. These studies reveal that the average intensity distribution at the receiver plane presents a central dark hollow profile, which is suitable for power coupling by the Cassegrain telescope receiver. In the optical system with optimized parameters, power coupling efficiency can keep in high values with the increase of the propagation distance. Under the atmospheric turbulent conditions, great advantages of vortex beam in power coupling of the two-Cassegrain-telescope optical system are shown in comparison with beam without vortex.

A New Metric for Land-Atmosphere Coupling Strength: Applications on Observations and Modeling

NASA Astrophysics Data System (ADS)

Tang, Q.; Xie, S.; Zhang, Y.; Phillips, T. J.; Santanello, J. A., Jr.; Cook, D. R.; Riihimaki, L.; Gaustad, K.

2017-12-01

A new metric is proposed to quantify the land-atmosphere (LA) coupling strength and is elaborated by correlating the surface evaporative fraction and impacting land and atmosphere variables (e.g., soil moisture, vegetation, and radiation). Based upon multiple linear regression, this approach simultaneously considers multiple factors and thus represents complex LA coupling mechanisms better than existing single variable metrics. The standardized regression coefficients quantify the relative contributions from individual drivers in a consistent manner, avoiding the potential inconsistency in relative influence of conventional metrics. Moreover, the unique expendable feature of the new method allows us to verify and explore potentially important coupling mechanisms. Our observation-based application of the new metric shows moderate coupling with large spatial variations at the U.S. Southern Great Plains. The relative importance of soil moisture vs. vegetation varies by location. We also show that LA coupling strength is generally underestimated by single variable methods due to their incompleteness. We also apply this new metric to evaluate the representation of LA coupling in the Accelerated Climate Modeling for Energy (ACME) V1 Contiguous United States (CONUS) regionally refined model (RRM). This work is performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. LLNL-ABS-734201

The role of ecosystem-atmosphere interactions in simulated Amazonian precipitation decrease and forest dieback under global climate warming

NASA Astrophysics Data System (ADS)

Betts, R. A.; Cox, P. M.; Collins, M.; Harris, P. P.; Huntingford, C.; Jones, C. D.

A suite of simulations with the HadCM3LC coupled climate-carbon cycle model is used to examine the various forcings and feedbacks involved in the simulated precipitation decrease and forest dieback. Rising atmospheric CO2 is found to contribute 20% to the precipitation reduction through the physiological forcing of stomatal closure, with 80% of the reduction being seen when stomatal closure was excluded and only radiative forcing by CO2 was included. The forest dieback exerts two positive feedbacks on the precipitation reduction; a biogeophysical feedback through reduced forest cover suppressing local evaporative water recycling, and a biogeochemical feedback through the release of CO2 contributing to an accelerated global warming. The precipitation reduction is enhanced by 20% by the biogeophysical feedback, and 5% by the carbon cycle feedback from the forest dieback. This analysis helps to explain why the Amazonian precipitation reduction simulated by HadCM3LC is more extreme than that simulated in other GCMs; in the fully-coupled, climate-carbon cycle simulation, approximately half of the precipitation reduction in Amazonia is attributable to a combination of physiological forcing and biogeophysical and global carbon cycle feedbacks, which are generally not included in other GCM simulations of future climate change. The analysis also demonstrates the potential contribution of regional-scale climate and ecosystem change to uncertainties in global CO2 and climate change projections. Moreover, the importance of feedbacks suggests that a human-induced increase in forest vulnerability to climate change may have implications for regional and global scale climate sensitivity.

Spatio-temporal dynamics of hydrographic reorganizations and iceberg discharges at the junction between the Northeast Atlantic and Norwegian Sea basins surrounding Heinrich event 4

NASA Astrophysics Data System (ADS)

Wary, Mélanie; Eynaud, Frédérique; Kissel, Catherine; Londeix, Laurent; Rossignol, Linda; Lapuyade, Joanna; Castéra, Marie-Hélène; Billy, Isabelle

2018-01-01

Dansgaard-Oeschger and Heinrich events constitute ones of the most enigmatic features of the last glacial period. Many studies have focused on their characteristic millennial climatic variability, testing atmospheric/cryospheric/oceanic couplings, but major uncertainties and discrepancies still remain. A new scenario, robustly supported by an approach coupling paleoreconstructions and freshwater hosing experiments simulating Heinrich-type perturbations, has recently emerged. Reconciling most of the up to now hypothesized theories, it suggests the occurrence of a regional seesaw between a cooled-down North Atlantic Ocean and warmed-up Nordic Seas during cold atmospheric phases, in relation to enhanced subsurface advection of warm Atlantic waters re-emerging in the Norwegian Sea. The associated ocean warming, thus reaching Nordic basins at a critical location beyond the Faeroe-Shetland sill, is proposed to be involved in the concomitant release of European icebergs. Here we further investigate this promising scenario over the 35-41 ka BP interval by (i) outlining its precise spatial pattern in a crucial area, i.e. the junction between the North Atlantic and the Norwegian Sea close to European ice-sheets, (ii) resolving its very fine temporal and regional evolution during critical transitions associated with the onset of warm advection, i.e. Greenland Interstadial to Greenland Stadial and Greenland Interstadial to Heinrich Stadial, and (iii) assessing its impact on the spatio-temporal dynamic of iceberg discharges from the European and Laurentide ice-sheets during cold stadial episodes especially including Heinrich event 4.

Experimental Insights into the Mechanisms of Particle Acceleration by Shock Waves

NASA Astrophysics Data System (ADS)

Scolamacchia, T.; Scheu, B.; Dingwell, D. B.

2011-12-01

The generation of shock waves is common during explosive volcanic eruptions. Particles acceleration following shock wave propagation has been experimentally observed suggesting the potential hazard related to this phenomenon. Experiments and numerical models focused on the dynamics of formation and propagation of different types of shock waves when overpressurized eruptive mixtures are suddenly released in the atmosphere, using a pseudo-gas approximation to model those mixtures. Nevertheless, the results of several studies indicated that the mechanism of coupling between a gas and solid particles is valid for a limited grain-size range, which at present is not well defined. We are investigating particle acceleration mechanisms using a vertical shock tube consisting of a high-pressure steel autoclave (450 mm long, 28 mm in diameter), pressurized with argon, and a low-pressure 140 mm long acrylic glass autoclave, with the same internal diameter of the HP reservoir. Shock waves are generated by Ar decompression at atmospheric pressures at Pres/Pamb 100:1 to 150:1, through the failure of a diaphragm. Experiments were performed either with empty autoclave or suspending solid analogue particles 150 μm in size inside the LP autoclave. Incident Mach number varied from 1.7 to 2.1. Absolute and relative pressure sensors monitored P histories during the entire process, and a high-speed camera recorded particles movement at 20,000 to 30,000 fps. Preliminary results indicate pressure multiplication at the contact between shock waves and the particles in a time lapse of 100s μs, suggesting a possible different mechanism with respect to gas-particle coupling for particle acceleration.

IPSL-CM5A2. An Earth System Model designed to run long simulations for past and future climates.

NASA Astrophysics Data System (ADS)

Sepulchre, Pierre; Caubel, Arnaud; Marti, Olivier; Hourdin, Frédéric; Dufresne, Jean-Louis; Boucher, Olivier

2017-04-01

The IPSL-CM5A model was developed and released in 2013 "to study the long-term response of the climate system to natural and anthropogenic forcings as part of the 5th Phase of the Coupled Model Intercomparison Project (CMIP5)" [Dufresne et al., 2013]. Although this model also has been used for numerous paleoclimate studies, a major limitation was its computation time, which averaged 10 model-years / day on 32 cores of the Curie supercomputer (on TGCC computing center, France). Such performances were compatible with the experimental designs of intercomparison projects (e.g. CMIP, PMIP) but became limiting for modelling activities involving several multi-millenial experiments, which are typical for Quaternary or "deeptime" paleoclimate studies, in which a fully-equilibrated deep-ocean is mandatory. Here we present the Earth-System model IPSL-CM5A2. Based on IPSL-CM5A, technical developments have been performed both on separate components and on the coupling system in order to speed up the whole coupled model. These developments include the integration of hybrid parallelization MPI-OpenMP in LMDz atmospheric component, the use of a new input-ouput library to perform parallel asynchronous input/output by using computing cores as "IO servers", the use of a parallel coupling library between the ocean and the atmospheric components. Running on 304 cores, the model can now simulate 55 years per day, opening new gates towards multi-millenial simulations. Apart from obtaining better computing performances, one aim of setting up IPSL-CM5A2 was also to overcome the cold bias depicted in global surface air temperature (t2m) in IPSL-CM5A. We present the tuning strategy to overcome this bias as well as the main characteristics (including biases) of the pre-industrial climate simulated by IPSL-CM5A2. Lastly, we shortly present paleoclimate simulations run with this model, for the Holocene and for deeper timescales in the Cenozoic, for which the particular continental configuration was overcome by a new design of the ocean tripolar grid.

Massive impact-induced release of carbon and sulfur gases in the early Earth's atmosphere

NASA Astrophysics Data System (ADS)

Marchi, S.; Black, B. A.; Elkins-Tanton, L. T.; Bottke, W. F.

2016-09-01

Recent revisions to our understanding of the collisional history of the Hadean and early-Archean Earth indicate that large collisions may have been an important geophysical process. In this work we show that the early bombardment flux of large impactors (>100 km) facilitated the atmospheric release of greenhouse gases (particularly CO2) from Earth's mantle. Depending on the timescale for the drawdown of atmospheric CO2, the Earth's surface could have been subject to prolonged clement surface conditions or multiple freeze-thaw cycles. The bombardment also delivered and redistributed to the surface large quantities of sulfur, one of the most important elements for life. The stochastic occurrence of large collisions could provide insights on why the Earth and Venus, considered Earth's twin planet, exhibit radically different atmospheres.

Contribution of tropical instability waves to ENSO irregularity

NASA Astrophysics Data System (ADS)

Holmes, Ryan M.; McGregor, Shayne; Santoso, Agus; England, Matthew H.

2018-05-01

Tropical instability waves (TIWs) are a major source of internally-generated oceanic variability in the equatorial Pacific Ocean. These non-linear phenomena play an important role in the sea surface temperature (SST) budget in a region critical for low-frequency modes of variability such as the El Niño-Southern Oscillation (ENSO). However, the direct contribution of TIW-driven stochastic variability to ENSO has received little attention. Here, we investigate the influence of TIWs on ENSO using a 1/4° ocean model coupled to a simple atmosphere. The use of a simple atmosphere removes complex intrinsic atmospheric variability while allowing the dominant mode of air-sea coupling to be represented as a statistical relationship between SST and wind stress anomalies. Using this hybrid coupled model, we perform a suite of coupled ensemble forecast experiments initiated with wind bursts in the western Pacific, where individual ensemble members differ only due to internal oceanic variability. We find that TIWs can induce a spread in the forecast amplitude of the Niño 3 SST anomaly 6-months after a given sequence of WWBs of approximately ± 45% the size of the ensemble mean anomaly. Further, when various estimates of stochastic atmospheric forcing are added, oceanic internal variability is found to contribute between about 20% and 70% of the ensemble forecast spread, with the remainder attributable to the atmospheric variability. While the oceanic contribution to ENSO stochastic forcing requires further quantification beyond the idealized approach used here, our results nevertheless suggest that TIWs may impact ENSO irregularity and predictability. This has implications for ENSO representation in low-resolution coupled models.

Validation of a Statistical Methodology for Extracting Vegetation Feedbacks: Focus on North African Ecosystems in the Community Earth System Model

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yu, Yan; Notaro, Michael; Wang, Fuyao

Generalized equilibrium feedback assessment (GEFA) is a potentially valuable multivariate statistical tool for extracting vegetation feedbacks to the atmosphere in either observations or coupled Earth system models. The reliability of GEFA at capturing the terrestrial impacts on regional climate is demonstrated in this paper using the National Center for Atmospheric Research Community Earth System Model (CESM), with focus on North Africa. The feedback is assessed statistically by applying GEFA to output from a fully coupled control run. To reduce the sampling error caused by short data records, the traditional or full GEFA is refined through stepwise GEFA by dropping unimportantmore » forcings. Two ensembles of dynamical experiments are developed for the Sahel or West African monsoon region against which GEFA-based vegetation feedbacks are evaluated. In these dynamical experiments, regional leaf area index (LAI) is modified either alone or in conjunction with soil moisture, with the latter runs motivated by strong regional soil moisture–LAI coupling. Stepwise GEFA boasts higher consistency between statistically and dynamically assessed atmospheric responses to land surface anomalies than full GEFA, especially with short data records. GEFA-based atmospheric responses are more consistent with the coupled soil moisture–LAI experiments, indicating that GEFA is assessing the combined impacts of coupled vegetation and soil moisture. Finally, both the statistical and dynamical assessments reveal a negative vegetation–rainfall feedback in the Sahel associated with an atmospheric stability mechanism in CESM versus a weaker positive feedback in the West African monsoon region associated with a moisture recycling mechanism in CESM.« less

Validation of a Statistical Methodology for Extracting Vegetation Feedbacks: Focus on North African Ecosystems in the Community Earth System Model

DOE PAGES

Yu, Yan; Notaro, Michael; Wang, Fuyao; ...

2018-02-05

Generalized equilibrium feedback assessment (GEFA) is a potentially valuable multivariate statistical tool for extracting vegetation feedbacks to the atmosphere in either observations or coupled Earth system models. The reliability of GEFA at capturing the terrestrial impacts on regional climate is demonstrated in this paper using the National Center for Atmospheric Research Community Earth System Model (CESM), with focus on North Africa. The feedback is assessed statistically by applying GEFA to output from a fully coupled control run. To reduce the sampling error caused by short data records, the traditional or full GEFA is refined through stepwise GEFA by dropping unimportantmore » forcings. Two ensembles of dynamical experiments are developed for the Sahel or West African monsoon region against which GEFA-based vegetation feedbacks are evaluated. In these dynamical experiments, regional leaf area index (LAI) is modified either alone or in conjunction with soil moisture, with the latter runs motivated by strong regional soil moisture–LAI coupling. Stepwise GEFA boasts higher consistency between statistically and dynamically assessed atmospheric responses to land surface anomalies than full GEFA, especially with short data records. GEFA-based atmospheric responses are more consistent with the coupled soil moisture–LAI experiments, indicating that GEFA is assessing the combined impacts of coupled vegetation and soil moisture. Finally, both the statistical and dynamical assessments reveal a negative vegetation–rainfall feedback in the Sahel associated with an atmospheric stability mechanism in CESM versus a weaker positive feedback in the West African monsoon region associated with a moisture recycling mechanism in CESM.« less

The Role of the Indian Ocean Sector for Prediction of the Coupled Indo-Pacific System: Impact of Atmospheric Coupling

NASA Technical Reports Server (NTRS)

Hackert, E. C.; Busalacchi, A. J.; Carton, J.; Murtugudde, R.; Arkin, P.; Evans, M. N.

2017-01-01

Indian Ocean (IO) dynamics impact ENSO predictability by influencing wind and precipitation anomalies in the Pacific. To test if the upstream influence of the IO improves ENSO validation statistics, a combination of forced ocean, atmosphere, and coupled models are utilized. In one experiment, the full tropical Indo-Pacific region atmosphere is forced by observed interannual SST anomalies. In the other, the IO is forced by climatological SST. Differences between these two forced atmospheric model experiments spotlight a much richer wind response pattern in the Pacific than previous studies that used idealized forcing and simple linear atmospheric models. Weak westerlies are found near the equator similar to earlier literature. However, at initialization strong easterlies between 30 deg. S to 10 deg. S and 0 deg. N to 25 deg. N and equatorial convergence of the meridional winds across the entire Pacific are unique findings from this paper. The large-scale equatorial divergence west of the dateline and northeasterly-to-northwesterly cross-equatorial flow converging on the equator east of the dateline in the Pacific are generated from interannual IO SST coupling. In addition, off-equatorial downwelling curl impacts large-scale oceanic waves (i.e., Rossby waves reflect as western boundary Kelvin waves). After 3 months, these downwelling equatorial Kelvin waves propagate across the Pacific and strengthen the NINO3 SST. Eventually Bjerknes feedbacks take hold in the eastern Pacific which allows this warm anomaly to grow. Coupled forecasts for NINO3 SST anomalies for 1993-2014 demonstrate that including interannual IO forcing significantly improves predictions for 3-9 month lead times.

The role of the Indian Ocean sector for prediction of the coupled Indo-Pacific system: Impact of atmospheric coupling

NASA Astrophysics Data System (ADS)

Hackert, E. C.; Busalacchi, A. J.; Carton, J.; Murtugudde, R.; Arkin, P.; Evans, M. N.

2017-04-01

Indian Ocean (IO) dynamics impact ENSO predictability by influencing wind and precipitation anomalies in the Pacific. To test if the upstream influence of the IO improves ENSO validation statistics, a combination of forced ocean, atmosphere, and coupled models are utilized. In one experiment, the full tropical Indo-Pacific region atmosphere is forced by observed interannual SST anomalies. In the other, the IO is forced by climatological SST. Differences between these two forced atmospheric model experiments spotlight a much richer wind response pattern in the Pacific than previous studies that used idealized forcing and simple linear atmospheric models. Weak westerlies are found near the equator similar to earlier literature. However, at initialization strong easterlies between 30°S-10°S and 0°N-25°N and equatorial convergence of the meridional winds across the entire Pacific are unique findings from this paper. The large-scale equatorial divergence west of the dateline and northeasterly-to-northwesterly cross-equatorial flow converging on the equator east of the dateline in the Pacific are generated from interannual IO SST coupling. In addition, off-equatorial downwelling curl impacts large-scale oceanic waves (i.e., Rossby waves reflect as western boundary Kelvin waves). After 3 months, these downwelling equatorial Kelvin waves propagate across the Pacific and strengthen the NINO3 SST. Eventually Bjerknes feedbacks take hold in the eastern Pacific which allows this warm anomaly to grow. Coupled forecasts for NINO3 SST anomalies for 1993-2014 demonstrate that including interannual IO forcing significantly improves predictions for 3-9 month lead times.

Verification and Validation of COAMPS: Results from a Fully-Coupled Air/Sea/Wave Modeling System

NASA Astrophysics Data System (ADS)

Smith, T.; Allard, R. A.; Campbell, T. J.; Chu, Y. P.; Dykes, J.; Zamudio, L.; Chen, S.; Gabersek, S.

2016-02-01

The Coupled Ocean/Atmosphere Mesoscale Prediction System (COAMPS) is a state-of-the art, fully-coupled air/sea/wave modeling system that is currently being validated for operational transition to both the Naval Oceanographic Office (NAVO) and to the Fleet Numerical Meteorology and Oceanography Center (FNMOC). COAMPS is run at the Department of Defense Supercomputing Resource Center (DSRC) operated by the DoD High Performance Computing Modernization Program (HPCMP). A total of four models including the Naval Coastal Ocean Model (NCOM), Simulating Waves Nearshore (SWAN), WaveWatch III, and the COAMPS atmospheric model are coupled through both the Earth System Modeling Framework (ESMF). Results from regions of naval operational interests, including the Western Atlantic (U.S. East Coast), RIMPAC (Hawaii), and DYNAMO (Indian Ocean), will show the advantages of utilizing a coupled modeling system versus an uncoupled or stand alone model. Statistical analyses, which include model/observation comparisons, will be presented in the form of operationally approved scorecards for both the atmospheric and oceanic output. Also, computational logistics involving the HPC resources for the COAMPS simulations will be shown.

High Order Accurate Finite Difference Modeling of Seismo-Acoustic Wave Propagation in a Moving Atmosphere and a Heterogeneous Earth Model Coupled Across a Realistic Topography

DOE Office of Scientific and Technical Information (OSTI.GOV)

Petersson, N. Anders; Sjogreen, Bjorn

Here, we develop a numerical method for simultaneously simulating acoustic waves in a realistic moving atmosphere and seismic waves in a heterogeneous earth model, where the motions are coupled across a realistic topography. We model acoustic wave propagation by solving the linearized Euler equations of compressible fluid mechanics. The seismic waves are modeled by the elastic wave equation in a heterogeneous anisotropic material. The motion is coupled by imposing continuity of normal velocity and normal stresses across the topographic interface. Realistic topography is resolved on a curvilinear grid that follows the interface. The governing equations are discretized using high ordermore » accurate finite difference methods that satisfy the principle of summation by parts. We apply the energy method to derive the discrete interface conditions and to show that the coupled discretization is stable. The implementation is verified by numerical experiments, and we demonstrate a simulation of coupled wave propagation in a windy atmosphere and a realistic earth model with non-planar topography.« less

High Order Accurate Finite Difference Modeling of Seismo-Acoustic Wave Propagation in a Moving Atmosphere and a Heterogeneous Earth Model Coupled Across a Realistic Topography

DOE PAGES

Petersson, N. Anders; Sjogreen, Bjorn

2017-04-18

Here, we develop a numerical method for simultaneously simulating acoustic waves in a realistic moving atmosphere and seismic waves in a heterogeneous earth model, where the motions are coupled across a realistic topography. We model acoustic wave propagation by solving the linearized Euler equations of compressible fluid mechanics. The seismic waves are modeled by the elastic wave equation in a heterogeneous anisotropic material. The motion is coupled by imposing continuity of normal velocity and normal stresses across the topographic interface. Realistic topography is resolved on a curvilinear grid that follows the interface. The governing equations are discretized using high ordermore » accurate finite difference methods that satisfy the principle of summation by parts. We apply the energy method to derive the discrete interface conditions and to show that the coupled discretization is stable. The implementation is verified by numerical experiments, and we demonstrate a simulation of coupled wave propagation in a windy atmosphere and a realistic earth model with non-planar topography.« less

The influence of oceanic basins on drought and ecosystem dynamics in Northeast Brazil

NASA Astrophysics Data System (ADS)

Santos Pereira, Marcos Paulo; Justino, Flavio; Mendes Malhado, Ana Claudia; Barbosa, Humberto; Marengo, José

2014-12-01

The 2012 drought in Northeast Brazil was the harshest in decades, with potentially significant impacts on the vegetation of the unique semi-arid caatinga biome and on local livelihoods. Here, we use a coupled climate-vegetation model (CCM3-IBIS) to: (1) investigate the role of the Pacific and Atlantic oceans in the 2012 drought, and; (2) evaluate the response of the caatinga vegetation to the 2012 climate extreme. Our results indicate that anomalous sea surface temperatures (SSTs) in the Atlantic Ocean were the primary factor forcing the 2012 drought, with Pacific Ocean SST having a larger role in sustaining typical climatic conditions in the region. The drought strongly influenced net primary production in the caatinga, causing a reduction in annual net ecosystem exchange indicating a reduction in amount of CO2 released to the atmosphere.

Effects of ocean-atmosphere coupling on rainfall over the Indian Ocean and northwestern Pacific Ocean during boreal summer

NASA Astrophysics Data System (ADS)

Zhou, Z. Q.; Xie, S. P.; Zhou, W.

2016-12-01

Atmosphere general circulation model (AGCM), forced with specified SST, has been widely used in climate studies. On one hand, AGCM is much faster to run compared to coupled general circulation model (CGCM). Also, the identical SST forcing allows a clean evaluation of the atmospheric component of CGCM. On the other hand, the coupling between atmosphere and ocean is missed in such atmosphere-only simulations. It is not clear how such simplification could affect the simulate of the atmosphere. In this study, the impact of ocean-atmosphere coupling is studied by comparing a CGCM simulation with an AGCM simulation which is forced with monthly SSTs specified from the CGCM simulation. Particularly, we focus on the climatology and interannual variability of rainfall over the IONWP during boreal summer. The IONWP is a unique region with a strong negative correlation between sea surface temperature (SST) and rainfall during boreal summer on the interannual time scale. The lead/lag correlation analysis suggests a negative feedback of rainfall on SST, which is only reasonably captured by CGCMs. We find that the lack of the negative feedback in AGCM not only enhances the climatology and interannual variability of rainfall but also increases the internal variability of rainfall over the IONWP. A simple mechanism is proposed to explain such enhancement. In addition, AGCM is able to capture the large-scale rainfall pattern over the IONWP during boreal summer, this is because that rainfall here is caused by remote ENSO effect on the interannual time scale. Our results herein suggest that people should be more careful when using an AGCM for climate change studies.

Assessing uncertainty and sensitivity of model parameterizations and parameters in WRF affecting simulated surface fluxes and land-atmosphere coupling over the Amazon region

NASA Astrophysics Data System (ADS)

Qian, Y.; Wang, C.; Huang, M.; Berg, L. K.; Duan, Q.; Feng, Z.; Shrivastava, M. B.; Shin, H. H.; Hong, S. Y.

2016-12-01

This study aims to quantify the relative importance and uncertainties of different physical processes and parameters in affecting simulated surface fluxes and land-atmosphere coupling strength over the Amazon region. We used two-legged coupling metrics, which include both terrestrial (soil moisture to surface fluxes) and atmospheric (surface fluxes to atmospheric state or precipitation) legs, to diagnose the land-atmosphere interaction and coupling strength. Observations made using the Department of Energy's Atmospheric Radiation Measurement (ARM) Mobile Facility during the GoAmazon field campaign together with satellite and reanalysis data are used to evaluate model performance. To quantify the uncertainty in physical parameterizations, we performed a 120 member ensemble of simulations with the WRF model using a stratified experimental design including 6 cloud microphysics, 3 convection, 6 PBL and surface layer, and 3 land surface schemes. A multiple-way analysis of variance approach is used to quantitatively analyze the inter- and intra-group (scheme) means and variances. To quantify parameter sensitivity, we conducted an additional 256 WRF simulations in which an efficient sampling algorithm is used to explore the multiple-dimensional parameter space. Three uncertainty quantification approaches are applied for sensitivity analysis (SA) of multiple variables of interest to 20 selected parameters in YSU PBL and MM5 surface layer schemes. Results show consistent parameter sensitivity across different SA methods. We found that 5 out of 20 parameters contribute more than 90% total variance, and first-order effects dominate comparing to the interaction effects. Results of this uncertainty quantification study serve as guidance for better understanding the roles of different physical processes in land-atmosphere interactions, quantifying model uncertainties from various sources such as physical processes, parameters and structural errors, and providing insights for improving the model physics parameterizations.

Interfacing a one-dimensional lake model with a single-column atmospheric model: 2. Thermal response of the deep Lake Geneva, Switzerland under a 2 × CO2 global climate change

NASA Astrophysics Data System (ADS)

Perroud, Marjorie; Goyette, StéPhane

2012-06-01

In the companion to the present paper, the one-dimensional k-ɛ lake model SIMSTRAT is coupled to a single-column atmospheric model, nicknamed FIZC, and an application of the coupled model to the deep Lake Geneva, Switzerland, is described. In this paper, the response of Lake Geneva to global warming caused by an increase in atmospheric carbon dioxide concentration (i.e., 2 × CO2) is investigated. Coupling the models allowed for feedbacks between the lake surface and the atmosphere and produced changes in atmospheric moisture and cloud cover that further modified the downward radiation fluxes. The time evolution of atmospheric variables as well as those of the lake's thermal profile could be reproduced realistically by devising a set of adjustable parameters. In a "control" 1 × CO2 climate experiment, the coupled FIZC-SIMSTRAT model demonstrated genuine skills in reproducing epilimnetic and hypolimnetic temperatures, with annual mean errors and standard deviations of 0.25°C ± 0.25°C and 0.3°C ± 0.15°C, respectively. Doubling the CO2 concentration induced an atmospheric warming that impacted the lake's thermal structure, increasing the stability of the water column and extending the stratified period by 3 weeks. Epilimnetic temperatures were seen to increase by 2.6°C to 4.2°C, while hypolimnion temperatures increased by 2.2°C. Climate change modified components of the surface energy budget through changes mainly in air temperature, moisture, and cloud cover. During summer, reduced cloud cover resulted in an increase in the annual net solar radiation budget. A larger water vapor deficit at the air-water interface induced a cooling effect in the lake.

Dynamics of the CRRES barium releases in the magnetosphere

NASA Technical Reports Server (NTRS)

Fuselier, S. A.; Mende, S. B.; Geller, S. P.; Miller, M.; Hoffman, R. A.; Wygant, J. R.; Pongratz, M.; Meredith, N. P.; Anderson, R. R.

1994-01-01

The Combined Release and Radiation Effects Satellite (CRRES) G-2, G-3, and G-4 ionized and neutral barium cloud positions are triangulated from ground-based optical data. From the time history of the ionized cloud motion perpendicular to the magnetic field, the late time coupling of the ionized cloud with the collisionless ambient plasma in the magnetosphere is investigated for each of the releases. The coupling of the ionized clouds with the ambient medium is quantitatively consistent with predictions from theory in that the coupling time increases with increasing distance from the Earth. Quantitative comparison with simple theory for the couping time also yields reasonable agreement. Other effects not predicted by the theory are discussed in the context of the observations.

The ozone depletion potentials on halocarbons: Their dependence of calculation assumptions

NASA Technical Reports Server (NTRS)

Karol, Igor L.; Kiselev, Andrey A.

1994-01-01

The concept of Ozone Depletion Potential (ODP) is widely used in the evaluation of numerous halocarbons and of their replacement effects on ozone, but the methods, assumptions and conditions used in ODP calculations have not been analyzed adequately. In this paper a model study of effects on ozone of the instantaneous releases of various amounts of CH3CCl3 and of CHF2Cl (HCFC-22) for several compositions of the background atmosphere are presented, aimed at understanding connections of ODP values with the assumptions used in their calculations. To facilitate the ODP computation in numerous versions for the long time periods after their releases, the above rather short-lived gases and the one-dimensional radiative photochemical model of the global annually averaged atmospheric layer up to 50 km height are used. The variation of released gas global mass from 1 Mt to 1 Gt leads to ODP value increase with its stabilization close to the upper bound of this range in the contemporary atmosphere. The same variations are analyzed for conditions of the CFC-free atmosphere of 1960's and for the anthropogenically loaded atmosphere in the 21st century according to the known IPCC 'business as usual' scenario. Recommendations for proper ways of ODP calculations are proposed for practically important cases.

Modified ensemble Kalman filter for nuclear accident atmospheric dispersion: prediction improved and source estimated.

PubMed

Zhang, X L; Su, G F; Yuan, H Y; Chen, J G; Huang, Q Y

2014-09-15

Atmospheric dispersion models play an important role in nuclear power plant accident management. A reliable estimation of radioactive material distribution in short range (about 50 km) is in urgent need for population sheltering and evacuation planning. However, the meteorological data and the source term which greatly influence the accuracy of the atmospheric dispersion models are usually poorly known at the early phase of the emergency. In this study, a modified ensemble Kalman filter data assimilation method in conjunction with a Lagrangian puff-model is proposed to simultaneously improve the model prediction and reconstruct the source terms for short range atmospheric dispersion using the off-site environmental monitoring data. Four main uncertainty parameters are considered: source release rate, plume rise height, wind speed and wind direction. Twin experiments show that the method effectively improves the predicted concentration distribution, and the temporal profiles of source release rate and plume rise height are also successfully reconstructed. Moreover, the time lag in the response of ensemble Kalman filter is shortened. The method proposed here can be a useful tool not only in the nuclear power plant accident emergency management but also in other similar situation where hazardous material is released into the atmosphere. Copyright © 2014 Elsevier B.V. All rights reserved.

Predicting seed dispersal using a Lagrangian Stochastic Model

NASA Astrophysics Data System (ADS)

Hsieh, C. I.; Chen, C. W.; Su, M. D.

2017-12-01

Migration and expansion of a plant species are determined by longdistance dispersion (LDD). A more sophisticated mechanical dispersion model is needed for mimicking LDD of wind-driven seeds. This study simulated seed dispersion trajectories in canopy turbulence by using the Lagrangian stochastic dispersion model under varying atmospheric stabilities in conjunction with the effects of turbulent kinetic energy dissipation rate intermittency. The effects of friction velocity, seed release height, and seed terminal velocity were also studied. The results showed that both the unstable atmosphere and the inclusion of the dissipation rate intermittency in the model could increase seeds' LDD. The number of seeds that escape the canopy volume by dissipation intermittency is increased under unstable atmospheric conditions. As a result, more seeds can be transported a further distance. When dissipation intermittency is included under astrong unstable atmosphere, the peak location of dispersal kernel tends to be closer to the source. Contrasting this, under both neutral and stable conditions when LDD of both are similar, the peak location will be further away from the source. However higher friction velocity, higher seed release height, and lower seed terminal velocity will all increase the LDD of seeds irregardless of atmospheric conditions. The change of LDD due to change in friction velocity, seed release height, or the seed terminal velocity, would be heightened under unstable conditions

The Introduction of High-Throughput Experimentation Methods for Suzuki-Miyaura Coupling Reactions in University Education

ERIC Educational Resources Information Center

Hoogenboom, Richard; Meier, Michael A. R.; Schubert, Ulrich S.

2005-01-01

A laboratory project permits for the discussion of the reaction mechanism of the Suzuki-Miyaura coupling reaction. The practical part of the project makes the students familiar with working under inert atmosphere but if the appropriate equipment for working under inert atmosphere is not available in a laboratory, novel catalysts that do not…

Validation of coupled atmosphere-fire behavior models

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bossert, J.E.; Reisner, J.M.; Linn, R.R.

1998-12-31

Recent advances in numerical modeling and computer power have made it feasible to simulate the dynamical interaction and feedback between the heat and turbulence induced by wildfires and the local atmospheric wind and temperature fields. At Los Alamos National Laboratory, the authors have developed a modeling system that includes this interaction by coupling a high resolution atmospheric dynamics model, HIGRAD, with a fire behavior model, BEHAVE, to predict the spread of wildfires. The HIGRAD/BEHAVE model is run at very high resolution to properly resolve the fire/atmosphere interaction. At present, these coupled wildfire model simulations are computationally intensive. The additional complexitymore » of these models require sophisticated methods for assuring their reliability in real world applications. With this in mind, a substantial part of the research effort is directed at model validation. Several instrumented prescribed fires have been conducted with multi-agency support and participation from chaparral, marsh, and scrub environments in coastal areas of Florida and inland California. In this paper, the authors first describe the data required to initialize the components of the wildfire modeling system. Then they present results from one of the Florida fires, and discuss a strategy for further testing and improvement of coupled weather/wildfire models.« less

50 CFR 635.26 - Catch and release.

Code of Federal Regulations, 2013 CFR

2013-10-01

... 50 Wildlife and Fisheries 12 2013-10-01 2013-10-01 false Catch and release. 635.26 Section 635.26 Wildlife and Fisheries FISHERY CONSERVATION AND MANAGEMENT, NATIONAL OCEANIC AND ATMOSPHERIC ADMINISTRATION, DEPARTMENT OF COMMERCE ATLANTIC HIGHLY MIGRATORY SPECIES Management Measures § 635.26 Catch and release. (a...

Impact of methane flow through deformable lake sediments on atmospheric release

NASA Astrophysics Data System (ADS)

Scandella, B.; Juanes, R.

2010-12-01

Methane is a potent greenhouse gas that is generated geothermally and biologically in lake and ocean sediments. Free gas bubbles may escape oxidative traps and contribute more to the atmospheric source than dissolved methane, but the details of the methane release depend on the interactions between the multiple fluid phases and the deformable porous medium. We present a model and supporting laboratory experiments of methane release through “breathing” dynamic flow conduits that open in response to drops in the hydrostatic load on lake sediments, which has been validated against a high-resolution record of free gas flux and hydrostatic pressure in Upper Mystic Lake, MA. In contrast to previous linear elastic fracture mechanics analysis of gassy sediments, the evolution of gas transport in a deformable compliant sediment is presented within the framework of multiphase poroplasticity. Experiments address how strongly the mode and rate of gas flow, captured by our model, impacts the size of bubbles released into the water column. A bubble's size in turn determines how efficiently it transports methane to the atmosphere, and integrating this effect will be critical to improving estimates of the atmospheric methane source from lakes. Cross-sectional schematic of lake sediments showing two venting sites: one open at left and one closed at right. The vertical release of gas bubbles (red) at the open venting site creates a local pressure drop, which drives both bubble formation from the methane-rich pore water (higher concentrations shaded darker red) and lateral advection of dissolved methane (purple arrows). Even as bubbles in the open site escape, those at the closed site remain trapped.

GEOS S2S-2_1: GMAO's New High Resolution Seasonal Prediction System

NASA Technical Reports Server (NTRS)

Molod, Andrea; Akella, Santha; Andrews, Lauren; Barahona, Donifan; Borovikov, Anna; Chang, Yehui; Cullather, Richard; Hackert, Eric; Kovach, Robin; Koster, Randal;

Combined climate and carbon-cycle effects of large-scale deforestation

PubMed Central

Bala, G.; Caldeira, K.; Wickett, M.; Phillips, T. J.; Lobell, D. B.; Delire, C.; Mirin, A.

2007-01-01

The prevention of deforestation and promotion of afforestation have often been cited as strategies to slow global warming. Deforestation releases CO2 to the atmosphere, which exerts a warming influence on Earth's climate. However, biophysical effects of deforestation, which include changes in land surface albedo, evapotranspiration, and cloud cover also affect climate. Here we present results from several large-scale deforestation experiments performed with a three-dimensional coupled global carbon-cycle and climate model. These simulations were performed by using a fully three-dimensional model representing physical and biogeochemical interactions among land, atmosphere, and ocean. We find that global-scale deforestation has a net cooling influence on Earth's climate, because the warming carbon-cycle effects of deforestation are overwhelmed by the net cooling associated with changes in albedo and evapotranspiration. Latitude-specific deforestation experiments indicate that afforestation projects in the tropics would be clearly beneficial in mitigating global-scale warming, but would be counterproductive if implemented at high latitudes and would offer only marginal benefits in temperate regions. Although these results question the efficacy of mid- and high-latitude afforestation projects for climate mitigation, forests remain environmentally valuable resources for many reasons unrelated to climate. PMID:17420463

Combined climate and carbon-cycle effects of large-scale deforestation.

PubMed

Bala, G; Caldeira, K; Wickett, M; Phillips, T J; Lobell, D B; Delire, C; Mirin, A

2007-04-17

The prevention of deforestation and promotion of afforestation have often been cited as strategies to slow global warming. Deforestation releases CO(2) to the atmosphere, which exerts a warming influence on Earth's climate. However, biophysical effects of deforestation, which include changes in land surface albedo, evapotranspiration, and cloud cover also affect climate. Here we present results from several large-scale deforestation experiments performed with a three-dimensional coupled global carbon-cycle and climate model. These simulations were performed by using a fully three-dimensional model representing physical and biogeochemical interactions among land, atmosphere, and ocean. We find that global-scale deforestation has a net cooling influence on Earth's climate, because the warming carbon-cycle effects of deforestation are overwhelmed by the net cooling associated with changes in albedo and evapotranspiration. Latitude-specific deforestation experiments indicate that afforestation projects in the tropics would be clearly beneficial in mitigating global-scale warming, but would be counterproductive if implemented at high latitudes and would offer only marginal benefits in temperate regions. Although these results question the efficacy of mid- and high-latitude afforestation projects for climate mitigation, forests remain environmentally valuable resources for many reasons unrelated to climate.

GEOS S2S-2_1: The GMAO new high resolution Seasonal Prediction System

NASA Astrophysics Data System (ADS)

Molod, A.; Vikhliaev, Y. V.; Hackert, E. C.; Kovach, R. M.; Zhao, B.; Cullather, R. I.; Marshak, J.; Borovikov, A.; Li, Z.; Barahona, D.; Andrews, L. C.; Chang, Y.; Schubert, S. D.; Koster, R. D.; Suarez, M.; Akella, S.

2017-12-01

A new version of the modeling and analysis system used to produce subseasonalto seasonal forecasts has just been released by the NASA/Goddard GlobalModeling and Assimilation Office. The new version runs at higher atmospheric resolution (approximately 1/2 degree globally), contains a subtantially improvedmodel description of the cryosphere, and includes additional interactive earth system model components (aerosol model). In addition, the Ocean data assimilationsystem has been replaced with a Local Ensemble Transform Kalman Filter.Here will describe the new system, along with the plans for the future (GEOS S2S-3_0) which will include a higher resolution ocean model and more interactive earth system model components (interactive vegetation, biomass burning from fires). We will alsopresent results from a free-running coupled simulation with the new system and resultsfrom a series of retrospective seasonal forecasts.Results from retrospective forecasts show significant improvements in surface temperaturesover much of the northern hemisphere and a much improved prediction of sea ice extent in bothhemispheres. The precipitation forecast skill is comparable to previous S2S systems, andthe only tradeoff is an increased "double ITCZ", which is expected as we go to higher atmospheric resolution.

Future directions of meteorology related to air-quality research.

PubMed

Seaman, Nelson L

2003-06-01

Meteorology is one of the major factors contributing to air-pollution episodes. More accurate representation of meteorological fields has been possible in recent years through the use of remote sensing systems, high-speed computers and fine-mesh meteorological models. Over the next 5-20 years, better meteorological inputs for air quality studies will depend on making better use of a wealth of new remotely sensed observations in more advanced data assimilation systems. However, for fine mesh models to be successful, parameterizations used to represent physical processes must be redesigned to be more precise and better adapted for the scales at which they will be applied. Candidates for significant overhaul include schemes to represent turbulence, deep convection, shallow clouds, and land-surface processes. Improvements in the meteorological observing systems, data assimilation and modeling, coupled with advancements in air-chemistry modeling, will soon lead to operational forecasting of air quality in the US. Predictive capabilities can be expected to grow rapidly over the next decade. This will open the way for a number of valuable new services and strategies, including better warnings of unhealthy atmospheric conditions, event-dependent emissions restrictions, and now casting support for homeland security in the event of toxic releases into the atmosphere.

Combined Climate and Carbon-Cycle Effects of Large-Scale Deforestation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bala, G; Caldeira, K; Wickett, M

2006-10-17

The prevention of deforestation and promotion of afforestation have often been cited as strategies to slow global warming. Deforestation releases CO{sub 2} to the atmosphere, which exerts a warming influence on Earth's climate. However, biophysical effects of deforestation, which include changes in land surface albedo, evapotranspiration, and cloud cover also affect climate. Here we present results from several large-scale deforestation experiments performed with a three-dimensional coupled global carbon-cycle and climate model. These are the first such simulations performed using a fully three-dimensional model representing physical and biogeochemical interactions among land, atmosphere, and ocean. We find that global-scale deforestation has amore » net cooling influence on Earth's climate, since the warming carbon-cycle effects of deforestation are overwhelmed by the net cooling associated with changes in albedo and evapotranspiration. Latitude-specific deforestation experiments indicate that afforestation projects in the tropics would be clearly beneficial in mitigating global-scale warming, but would be counterproductive if implemented at high latitudes and would offer only marginal benefits in temperate regions. While these results question the efficacy of mid- and high-latitude afforestation projects for climate mitigation, forests remain environmentally valuable resources for many reasons unrelated to climate.« less

Biosphere-Atmosphere Transfer Scheme (BATS) version le as coupled to the NCAR community climate model. Technical note. [NCAR (National Center for Atmospheric Research)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dickinson, R.E.; Henderson-Sellers, A.; Kennedy, P.J.

A comprehensive model of land-surface processes has been under development suitable for use with various National Center for Atmospheric Research (NCAR) General Circulation Models (GCMs). Special emphasis has been given to describing properly the role of vegetation in modifying the surface moisture and energy budgets. The result of these efforts has been incorporated into a boundary package, referred to as the Biosphere-Atmosphere Transfer Scheme (BATS). The current frozen version, BATS1e is a piece of software about four thousand lines of code that runs as an offline version or coupled to the Community Climate Model (CCM).

Meridionally propagating interannual-to-interdecadal variability in a linear ocean-atmosphere model

NASA Technical Reports Server (NTRS)

Mehta, Vikram M.

1992-01-01

Meridional oscillation modes in a global, primitive-equation coupled ocean-atmosphere model have been analyzed in order to determine whether they contain such meridionally propagating modes as surface-pressure perturbations with years-to-decades oscillation periods. A two-layer global ocean model and a two-level global atmosphere model were then formulated. For realistic parameter values and basic states, meridional modes oscillating at periods of several years to several decades are noted to be present in the coupled ocean-atmosphere model; the oscillation periods, travel times, and meridional structures of surface pressure perturbations in one of the modes are found to be comparable to the corresponding characteristics of observed sea-level pressure perturbations.

Moistening of the northern North American Great Plains enhances land-atmosphere coupling

NASA Astrophysics Data System (ADS)

Gerken, T.; Bromley, G. T.; Stoy, P. C.

2017-12-01

Land use change impacts planetary boundary layer processes and regional climate by altering the magnitude and timing of water and energy flux into the atmosphere. In the North American Great Plains (NGP), a decline in the practice of summer fallow on the order of 20 Mha from the 1970s until the present has coincided with a decrease in summertime radiative forcing, on the order of 6 W m-2. MERRA 2 (Modern-Era Retrospective analysis for Research and Applications) for the area near Fort Peck, Montana, (a FLUXNET site established in 2000) shows a decrease of summertime (June-August) sensible heat fluxes ranging from -3.6 to -8.5 W m-2 decade-1, associated with an increase of latent heat fluxes (5.2-9.1 W m-2 decade-1) since the 1980s. Net radiation changed little. The result was a strong decrease of summer Bowen ratios from 1.5-2 in 1980 to approximately 1 in 2015. Findings are consistent with the effects on increased summertime evapotranspiration due to reduction in summer fallow that should lead to smaller Bowen ratios and a larger build-up of moist static energy. We use a mixed-layer (ML) atmospheric modeling framework to further investigate the impact of the surface energy balance on convective development and local land-atmosphere coupling in the NGP. Using summertime eddy covariance data from Fort Peck and atmospheric soundings from the nearby Glasgow airport, we compare the development of modeled ML and lifted condensation level (LCL) to find times of ML exceeding LCL, a necessary but not sufficient condition for the occurrence of convective precipitation. We establish that the ML model adequately captures ML heights and timing of locally triggered convection at the site and that there is a c. 10% increase in modeled convection permitting conditions today compared to 1975-85 in response to ML-moistening and decreasing Bo. We find that growing season land-atmosphere coupling develops from wet preference in May to dry coupling in July and atmospheric suppression of convection in September, highlighting the importance of subseasonal dynamics for precipitation. The approach is extended to the regional scale using fluxes and profiles from MERRA2 to establish the exact nature or land-atmosphere coupling associated with moistening of the atmospheric boundary-layer for the NGP region.

Taking the pulse of the carbon release during the onset of the Paleocene-Eocene thermal maximum

NASA Astrophysics Data System (ADS)

Babila, T. L.; Bralower, T. J.; Robinson, M. M.; Self-Trail, J. M.; Zachos, J. C.

2015-12-01

The Paleocene-Eocene thermal maximum (PETM) (~55 Ma) is a warming event characterized by a negative carbon isotope excursion (CIE) representing a large and rapid injection of carbon into global reservoirs. Debate continues regarding the mechanism, magnitude, and tempo of the carbon released. A few terrestrial and marine sediment records document two distinct δ13C excursions a pre-onset excursion (POE) and CIE interpreted as evidence of multiple carbon injections. We generated geochemical records of ocean carbonate chemistry and temperature using cores drilled by the U.S Geological Survey (USGS) that recovered expanded sections of the PETM onset along the mid-Atlantic coastal plain. Our stable isotope (δ13C and δ18O) planktonic foraminifer records from South Dover Bridge (SDB), Maryland USA exhibit prominent anomalies across the Paleocene-Eocene boundary consistent to proximal coastal sites. δ13C records of mixed-layer (Acarinina spp.) and thermocline (Subbotina spp.) dwelling planktonic foraminifera show two negative carbon excursions that include a 2 ‰ POE and 3-4 ‰ CIE that return to baseline values between events in conjunction with bulk carbonate trends. Remarkably, contemporaneous foraminifer δ18O records exhibit only a minor response during the POE. This could be an artifact of preservation, or at face value, indicative of little to no warming. For the latter, this would require a rapid, but relatively small carbon release. To test the coupled link between atmosphere and surface ocean δ13C records we aim to integrate our geochemical results with model simulations to establish the duration and global extent of multiple carbon releases.

Methane clathrate stability zone variations and gas transport in the Martian subsurface

NASA Astrophysics Data System (ADS)

Karatekin, O.; Gloesener, E.; Dehant, V. M. A.; Temel, O.

2016-12-01

During the last years, several detections of methane in the atmosphere of Mars were reported from Earth-based and Mars orbit instruments with abundances ranging to tens of parts-per-billion by volume (ppbv). Recently, the Curiosity rover detected methane with background levels of 0.7 ppbv and episodic releases of 7 ppbv. Although the methane sources are still unknown, this gas may have been stored in reservoirs of clathrate hydrate in the Martian subsurface where thermodynamics conditions are favourable to their presence. Clathrate hydrates are crystalline compounds constituted by cages formed by hydrogen-bonded water molecules inside of which guest gas molecules are trapped. In this study, methane clathrate stability in the Martian subsurface are investigated and their temporal and spatial variations are studied. Present-day maps of methane clathrate stability zone are produced by coupling the stability conditions of methane clathrate with a subsurface model using the available observations such as the the thermal inertia derived from TES MGS data. Then, a gas transport model has been used to study the methane flux at the surface due to the diffusion of different plausible methane volumes released by clathrate hydrates at variable depths under the Martian surface.

Predicting Coupled Ocean-Atmosphere Modes with a Climate Modeling Hierarchy -- Final Report

DOE Office of Scientific and Technical Information (OSTI.GOV)

Michael Ghil, UCLA; Andrew W. Robertson, IRI, Columbia Univ.; Sergey Kravtsov, U. of Wisconsin, Milwaukee

The goal of the project was to determine midlatitude climate predictability associated with tropical-extratropical interactions on interannual-to-interdecadal time scales. Our strategy was to develop and test a hierarchy of climate models, bringing together large GCM-based climate models with simple fluid-dynamical coupled ocean-ice-atmosphere models, through the use of advanced probabilistic network (PN) models. PN models were used to develop a new diagnostic methodology for analyzing coupled ocean-atmosphere interactions in large climate simulations made with the NCAR Parallel Climate Model (PCM), and to make these tools user-friendly and available to other researchers. We focused on interactions between the tropics and extratropics throughmore » atmospheric teleconnections (the Hadley cell, Rossby waves and nonlinear circulation regimes) over both the North Atlantic and North Pacific, and the ocean’s thermohaline circulation (THC) in the Atlantic. We tested the hypothesis that variations in the strength of the THC alter sea surface temperatures in the tropical Atlantic, and that the latter influence the atmosphere in high latitudes through an atmospheric teleconnection, feeding back onto the THC. The PN model framework was used to mediate between the understanding gained with simplified primitive equations models and multi-century simulations made with the PCM. The project team is interdisciplinary and built on an existing synergy between atmospheric and ocean scientists at UCLA, computer scientists at UCI, and climate researchers at the IRI.« less

Putting out the fire: what terminates calcium-induced calcium release in cardiac muscle?

PubMed

Stern, Michael D; Cheng, Heping

2004-06-01

The majority of contractile calcium in cardiac muscle is released from stores in the sarcoplasmic reticulum (SR), by a process of calcium-induced calcium release (CICR) through ryanodine receptors. Because CICR is intrinsically self-reinforcing, the stability of and graded regulation of cardiac EC coupling appear paradoxical. It is now well established that this gradation results from the stochastic recruitment of varying numbers of elementary local release events, which may themselves be regenerative, and which can be directly observed as calcium sparks. Ryanodine receptors (RyRs) are clustered in dense lattices, and most calcium sparks are now believed to involve activation of multiple RyRs. This implies that local CICR is regenerative, requiring a mechanism to terminate it. It was initially assumed that this mechanism was inactivation of the RyR, but during the decade since the discovery of sparks, no sufficiently strong inactivation mechanism has been demonstrated in vitro and all empirically determined gating schemes for the RyR give unstable EC coupling in Monte Carlo simulations. We consider here possible release termination mechanisms. Stochastic attrition is the spontaneous decay of active clusters due to random channel closure; calculations show that it is much too slow unless assisted by another process. Calcium-dependent RyR inactivation involving third-party proteins remains a viable but speculative mechanism; current candidates include calmodulin and sorcin. Local depletion of SR release terminal calcium could terminate release, however calculations and measurements leave it uncertain whether a sufficient diffusion resistance exists within the SR to sustain such depletion. Depletion could be assisted by dependence of RyR activity on SR lumenal [Ca(2+)]. There is substantial evidence for such lumenal activation, but it is not clear if it is a strong enough effect to account for the robust termination of sparks. The existence of direct interactions among clustered RyRs might account for the discrepancy between the inactivation properties of isolated RyRs and intact clusters. Such coupled gating remains controversial. Determining the mechanism of release termination is the outstanding unsolved problem of cardiac EC coupling, and will probably require extensive genetic manipulation of the EC coupling apparatus in its native environment to unravel the solution.

Assessing Extratropical Influence on Tropical Climatology and Variability with Regional Coupled Data Assimilation

NASA Astrophysics Data System (ADS)

Lu, F.; Liu, Z.; Liu, Y.; Zhang, S.; Jacob, R. L.

2017-12-01

The Regional Coupled Data Assimilation (RCDA) method is introduced as a tool to study coupled climate dynamics and teleconnections. The RCDA method is built on an ensemble-based coupled data assimilation (CDA) system in a coupled general circulation model (CGCM). The RCDA method limits the data assimilation to the desired model components (e.g. atmosphere) and regions (e.g. the extratropics), and studies the ensemble-mean model response (e.g. tropical response to "observed" extratropical atmospheric variability). When applied to the extratropical influence on tropical climate, the RCDA method has shown some unique advantages, namely the combination of a fully coupled model, real-world observations and an ensemble approach. Tropical variability (e.g. El Niño-Southern Oscillation or ENSO) and climatology (e.g. asymmetric Inter-Tropical Convergence Zone or ITCZ) were initially thought to be determined mostly by local forcing and ocean-atmosphere interaction in the tropics. Since late 20th century, numerous studies have showed that extratropical forcing could affect, or even largely determine some aspects of the tropical climate. Due to the coupled nature of the climate system, however, the challenge of determining and further quantifying the causality of extratropical forcing on the tropical climate remains. Using the RCDA method, we have demonstrated significant control of extratropical atmospheric forcing on ENSO variability in a CGCM, both with model-generated and real-world observation datasets. The RCDA method has also shown robust extratropical impact on the tropical double-ITCZ bias in a CGCM. The RCDA method has provided the first systematic and quantitative assessment of extratropical influence on tropical climatology and variability by incorporating real world observations in a CGCM.

Coupled atmosphere/canopy model for remote sensing of plant reflectance features

NASA Technical Reports Server (NTRS)

Gerstl, S. A.; Zardecki, A.

1985-01-01

Solar radiative transfer through a coupled system of atmosphere and plant canopy is modeled as a multiple-scattering problem through a layered medium of random scatterers. The radiative transfer equation is solved by the discrete-ordinates finite-element method. Analytic expressions are derived that allow the calculation of scattering and absorption cross sections for any plant canopy layer form measurable biophysical parameters such as the leaf area index, leaf angle distribution, and individual leaf reflectance and transmittance data. An expression for a canopy scattering phase function is also given. Computational results are in good agreement with spectral reflectance measurements directly above a soybean canopy, and the concept of greenness- and brightness-transforms of Landsat MSS data is reconfirmed with the computed results. A sensitivity analysis with the coupled atmosphere/canopy model quantifies how satellite-sensed spectral radiances are affected by increased atmospheric aerosols, by varying leaf area index, by anisotropic leaf scattering, and by non-Lambertian soil boundary conditions. Possible extensions to a 2-D model are also discussed.

On the Role of Dissolved Gases in the Atmosphere Retention of Low-mass Low-density Planets

NASA Astrophysics Data System (ADS)

Chachan, Yayaati; Stevenson, David J.

2018-02-01

Low-mass low-density planets discovered by Kepler in the super-Earth mass regime typically have large radii for their inferred masses, implying the presence of H2–He atmospheres. These planets are vulnerable to atmospheric mass loss due to heating by the parent star’s XUV flux. Models coupling atmospheric mass loss with thermal evolution predicted a bimodal distribution of planetary radii, which has gained observational support. However, a key component that has been ignored in previous studies is the dissolution of these gases into the molten core of rock and iron that constitute most of their mass. Such planets have high temperatures (>2000 K) and pressures (∼kbars) at the core-envelope boundary, ensuring a molten surface and a subsurface reservoir of hydrogen that can be 5–10 times larger than the atmosphere. This study bridges this gap by coupling the thermal evolution of the planet and the mass loss of the atmosphere with the thermodynamic equilibrium between the dissolved H2 and the atmospheric H2 (Henry’s law). Dissolution in the interior allows a planet to build a larger hydrogen repository during the planet formation stage. We show that the dissolved hydrogen outgasses to buffer atmospheric mass loss. The slow cooling of the planet also leads to outgassing because solubility decreases with decreasing temperature. Dissolution of hydrogen in the interior therefore increases the atmosphere retention ability of super-Earths. The study highlights the importance of including the temperature- and pressure-dependent solubility of gases in magma oceans and coupling outgassing to planetary evolution models.

Study of Atmospheric Forcing and Responses (SAFAR) campaign: overview

NASA Astrophysics Data System (ADS)

Jayaraman, A.; Venkat Ratnam, M.; Patra, A. K.; Narayana Rao, T.; Sridharan, S.; Rajeevan, M.; Gadhavi, H.; Kesarkar, A. P.; Srinivasulu, P.; Raghunath, K.

2010-01-01

Study of Atmospheric Forcing and Responses (SAFAR) is a five year (2009-2014) research programme specifically to address the responses of the earth's atmosphere to both natural and anthropogenic forcings using a host of collocated instruments operational at the National Atmospheric Research Laboratory, Gadanki (13.5° N, 79.2° E), India from a unified viewpoint of studying the vertical coupling between the forcings and responses from surface layer to the ionosphere. As a prelude to the main program a pilot campaign was conducted at Gadanki during May-November 2008 using collocated observations from the MST radar, Rayleigh lidar, GPS balloonsonde, and instruments measuring aerosol, radiation and precipitation, and supporting satellite data. We show the importance of the large radiative heating caused by absorption of solar radiation by soot particles in the lower atmosphere, the observed high vertical winds in the convective updrafts extending up to tropopause, and the difficulty in simulating the same with existing models, the upward traveling waves in the middle atmosphere coupling the lower atmosphere with the upper atmosphere, their manifestation in the mesospheric temperature structure and inversion layers, the mesopause height extending up to 100 km, and the electro-dynamical coupling between mesosphere and the ionosphere which causes irregularities in the ionospheric F-region. The purpose of this communication is not only to share the knowledge that we gained from the SAFAR pilot campaign, but also to inform the international atmospheric science community about the SAFAR program as well as to extend our invitation to join in our journey.

Experimental demonstration of single-mode fiber coupling over relatively strong turbulence with adaptive optics.

PubMed

Chen, Mo; Liu, Chao; Xian, Hao

2015-10-10

High-speed free-space optical communication systems using fiber-optic components can greatly improve the stability of the system and simplify the structure. However, propagation through atmospheric turbulence degrades the spatial coherence of the signal beam and limits the single-mode fiber (SMF) coupling efficiency. In this paper, we analyze the influence of the atmospheric turbulence on the SMF coupling efficiency over various turbulences. The results show that the SMF coupling efficiency drops from 81% without phase distortion to 10% when phase root mean square value equals 0.3λ. The simulations of SMF coupling with adaptive optics (AO) indicate that it is inevitable to compensate the high-order aberrations for SMF coupling over relatively strong turbulence. The SMF coupling efficiency experiments, using an AO system with a 137-element deformable mirror and a Hartmann-Shack wavefront sensor, obtain average coupling efficiency increasing from 1.3% in open loop to 46.1% in closed loop under a relatively strong turbulence, D/r₀=15.1.

Global seasonal climate predictability in a two tiered forecast system: part I: boreal summer and fall seasons

NASA Astrophysics Data System (ADS)

Misra, Vasubandhu; Li, H.; Wu, Z.; DiNapoli, S.

2014-03-01

This paper shows demonstrable improvement in the global seasonal climate predictability of boreal summer (at zero lead) and fall (at one season lead) seasonal mean precipitation and surface temperature from a two-tiered seasonal hindcast forced with forecasted SST relative to two other contemporary operational coupled ocean-atmosphere climate models. The results from an extensive set of seasonal hindcasts are analyzed to come to this conclusion. This improvement is attributed to: (1) The multi-model bias corrected SST used to force the atmospheric model. (2) The global atmospheric model which is run at a relatively high resolution of 50 km grid resolution compared to the two other coupled ocean-atmosphere models. (3) The physics of the atmospheric model, especially that related to the convective parameterization scheme. The results of the seasonal hindcast are analyzed for both deterministic and probabilistic skill. The probabilistic skill analysis shows that significant forecast skill can be harvested from these seasonal hindcasts relative to the deterministic skill analysis. The paper concludes that the coupled ocean-atmosphere seasonal hindcasts have reached a reasonable fidelity to exploit their SST anomaly forecasts to force such relatively higher resolution two tier prediction experiments to glean further boreal summer and fall seasonal prediction skill.

Advanced Atmospheric Ensemble Modeling Techniques

DOE Office of Scientific and Technical Information (OSTI.GOV)

Buckley, R.; Chiswell, S.; Kurzeja, R.

Ensemble modeling (EM), the creation of multiple atmospheric simulations for a given time period, has become an essential tool for characterizing uncertainties in model predictions. We explore two novel ensemble modeling techniques: (1) perturbation of model parameters (Adaptive Programming, AP), and (2) data assimilation (Ensemble Kalman Filter, EnKF). The current research is an extension to work from last year and examines transport on a small spatial scale (<100 km) in complex terrain, for more rigorous testing of the ensemble technique. Two different release cases were studied, a coastal release (SF6) and an inland release (Freon) which consisted of two releasemore » times. Observations of tracer concentration and meteorology are used to judge the ensemble results. In addition, adaptive grid techniques have been developed to reduce required computing resources for transport calculations. Using a 20- member ensemble, the standard approach generated downwind transport that was quantitatively good for both releases; however, the EnKF method produced additional improvement for the coastal release where the spatial and temporal differences due to interior valley heating lead to the inland movement of the plume. The AP technique showed improvements for both release cases, with more improvement shown in the inland release. This research demonstrated that transport accuracy can be improved when models are adapted to a particular location/time or when important local data is assimilated into the simulation and enhances SRNL’s capability in atmospheric transport modeling in support of its current customer base and local site missions, as well as our ability to attract new customers within the intelligence community.« less

Whole Atmosphere Modeling and Data Analysis: Success Stories, Challenges and Perspectives

NASA Astrophysics Data System (ADS)

Yudin, V. A.; Akmaev, R. A.; Goncharenko, L. P.; Fuller-Rowell, T. J.; Matsuo, T.; Ortland, D. A.; Maute, A. I.; Solomon, S. C.; Smith, A. K.; Liu, H.; Wu, Q.

2015-12-01

At the end of the 20-th century Raymond Roble suggested an ambitious target of developing an atmospheric general circulation model (GCM) that spans from the surface to the thermosphere for modeling the coupled atmosphere-ionosphere with drivers from terrestrial meteorology and solar-geomagnetic inputs. He pointed out several areas of research and applications that would benefit highly from the development and improvement of whole atmosphere modeling. At present several research groups using middle and whole atmosphere models have attempted to perform coupled ionosphere-thermosphere predictions to interpret the "unexpected" anomalies in the electron content, ions and plasma drifts observed during recent stratospheric warming events. The recent whole atmosphere inter-comparison case studies also displayed striking differences in simulations of prevailing flows, planetary waves and dominant tidal modes even when the lower atmosphere domain of those models were constrained by similar meteorological analyses. We will present the possible reasons of such differences between data-constrained whole atmosphere simulations when analyses with 6-hour time resolution are used and discuss the potential model-data and model-model differences above the stratopause. The possible shortcomings of the whole atmosphere simulations associated with model physics, dynamical cores and resolutions will be discussed. With the increased confidence in the space-borne temperature, winds and ozone observations and extensive collections of ground-based upper atmosphere observational facilities, the whole atmosphere modelers will be able to quantify annual and year-to-variability of the zonal mean flows, planetary wave and tides. We will demonstrate the value of tidal and planetary wave variability deduced from the space-borne data and ground-based systems for evaluation and tune-up of whole atmosphere simulations including corrections of systematic model errors. Several success stories on the middle and whole atmosphere simulations coupled with the ionosphere models will be highlighted, and future perspectives for links of the space and terrestrial weather predictions constrained by current and scheduled ionosphere-thermosphere-mesosphere satellite missions will be presented

The Community Climate System Model.

NASA Astrophysics Data System (ADS)

Blackmon, Maurice; Boville, Byron; Bryan, Frank; Dickinson, Robert; Gent, Peter; Kiehl, Jeffrey; Moritz, Richard; Randall, David; Shukla, Jagadish; Solomon, Susan; Bonan, Gordon; Doney, Scott; Fung, Inez; Hack, James; Hunke, Elizabeth; Hurrell, James; Kutzbach, John; Meehl, Jerry; Otto-Bliesner, Bette; Saravanan, R.; Schneider, Edwin K.; Sloan, Lisa; Spall, Michael; Taylor, Karl; Tribbia, Joseph; Washington, Warren

2001-11-01

The Community Climate System Model (CCSM) has been created to represent the principal components of the climate system and their interactions. Development and applications of the model are carried out by the U.S. climate research community, thus taking advantage of both wide intellectual participation and computing capabilities beyond those available to most individual U.S. institutions. This article outlines the history of the CCSM, its current capabilities, and plans for its future development and applications, with the goal of providing a summary useful to present and future users. The initial version of the CCSM included atmosphere and ocean general circulation models, a land surface model that was grafted onto the atmosphere model, a sea-ice model, and a flux coupler that facilitates information exchanges among the component models with their differing grids. This version of the model produced a successful 300-yr simulation of the current climate without artificial flux adjustments. The model was then used to perform a coupled simulation in which the atmospheric CO2 concentration increased by 1% per year. In this version of the coupled model, the ocean salinity and deep-ocean temperature slowly drifted away from observed values. A subsequent correction to the roughness length used for sea ice significantly reduced these errors. An updated version of the CCSM was used to perform three simulations of the twentieth century's climate, and several pro-jections of the climate of the twenty-first century. The CCSM's simulation of the tropical ocean circulation has been significantly improved by reducing the background vertical diffusivity and incorporating an anisotropic horizontal viscosity tensor. The meridional resolution of the ocean model was also refined near the equator. These changes have resulted in a greatly improved simulation of both the Pacific equatorial undercurrent and the surface countercurrents. The interannual variability of the sea surface temperature in the central and eastern tropical Pacific is also more realistic in simulations with the updated model. Scientific challenges to be addressed with future versions of the CCSM include realistic simulation of the whole atmosphere, including the middle and upper atmosphere, as well as the troposphere; simulation of changes in the chemical composition of the atmosphere through the incorporation of an integrated chemistry model; inclusion of global, prognostic biogeochemical components for land, ocean, and atmosphere; simulations of past climates, including times of extensive continental glaciation as well as times with little or no ice; studies of natural climate variability on seasonal-to-centennial timescales; and investigations of anthropogenic climate change. In order to make such studies possible, work is under way to improve all components of the model. Plans call for a new version of the CCSM to be released in 2002. Planned studies with the CCSM will require much more computer power than is currently available.

Use of spatially refined satellite remote sensing fire detection data to initialize and evaluate coupled weather-wildfire growth model simulations

NASA Astrophysics Data System (ADS)

Schroeder, W.; Coen, J.; Oliva, P.

2013-12-01

Availability of spatially refined satellite active fire detection data is gradually increasing. For example, the new 375 m Visible Infrared Imaging Radiometer Suite (VIIRS) data show improved active fire detection performance for both small and large size fires. The VIIRS data have proved superior to MODIS for mapping of wildfires events spanning several days to weeks of either continued or intermittent activity, delivering 12-h active fire data of improved spatial fidelity. The VIIRS active fire data are complemented by other satellite active fire data sets of similar or higher spatial resolution, including the new 30 m Landsat-8. Additional assets should include the upcoming 20 m Sentinel-2 Landsat-class satellite program by the European Space Agency to be launched in 2014-15. These improved active fire data sets are fostering new applications that rely on higher resolution input fire data. In this study, we describe the characteristics of the new VIIRS and Landsat-8 data and demonstrate one such new application of satellite active fire data in support of fire behavior modeling. We present results for a wildfire observed in June 2012 in New Mexico using an innovative approach to improving the simulation of large, long-duration wildfires, either for retrospective studies or forecasting in a number of geophysical applications. The approach uses (1) the Coupled Atmosphere-Wildland Fire Environment (CAWFE) Model, a numerical weather prediction model two-way coupled with a module representing the rate of spread of a wildfire's flaming front, its rate of consumption of different wildland fuels, and the feedback of this heat release upon the atmosphere - i.e. 'how a fire creates its own weather', combined with (2) spatially refined 375 m VIIRS active fire data, which is used for initialization of a wildfire already in progress in the model and evaluation of its simulated progression at the time of the next pass. Results show that initializing a fire that is 'in progress' with VIIRS data and a weather simulation based on more recent atmospheric analyses can overcome several issues and improve the simulation of late-developing fires and of later periods (particularly those with growth periods separated by lulls) in a long-lived fire.

Effect of Interactive River Routing on North Atlantic Overturning in a Simulation of the last Deglaciation

NASA Astrophysics Data System (ADS)

Mikolajewicz, Uwe; Ziemen, Florian; Kapsch, Marie; Meccia, Virna

2017-04-01

One of the major challenges in climate modeling is the simulation of glacial-interglacial transitions. A few models of intermediate complexity have been successful in simulating the last termination. Complex atmosphere-ocean general circulation models (AOGCMs) with prescribed ice sheets are able to yield realistic climate changes. Here we present results from our first attempt to simulate a substantial part of the last glacial cycle with an AOGCM coupled interactively with a state-of-the-art ice sheet model. The ECHAM5/MPIOM AOGCM is interactively coupled to the dynamical ice sheet model PISM and the dynamical vegetation model LPJ. The model is integrated from the late Glacial into the Holocene using insolation and greenhouse gas concentrations as transient forcing. To make the long simulations feasible, the atmosphere is accelerated by a factor of 10 relative to the other components using a periodical-synchronous coupling technique. The land sea mask remains fixed at the LGM state. River routing and surface elevation are calculated interactively. A mini-ensemble with different initial conditions is performed. Additionally, one fully synchronously simulation, without acceleration in the atmosphere, is run. In all simulations the northern hemisphere deglaciation starts between 18 and 17 kyr BP, consistent with the onset of global warming. The model produces Heinrich event like variability. These rapid ice discharge events have a strong impact on the North Atlantic meridional overturning circulation (NAMOC). The interactive river routing has a strong impact on the simulated NAMOC during the deglaciation. The retreat of the Laurentide Ice Sheet together with the depressed topography due to the former ice load leads to a redirection of the river routes.. In particular, the discharge route for runoff from the melting southwestern Laurentide shifts from the Gulf of Mexico to the Arctic. The consequence is a rapid reduction/suppression of the North Atlantic deep water (NADW) formation. When the Laurentide Ice Sheet retreats from the Hudson Strait, this becomes the new drainage route. Hence, fresh water is released into the Labrador Sea and is less effective in suppressing the deep water formation in the North Atlantic. As a consequence, the NADW formation recovers within a few decades. Our results show the potential importance of interactive river routing for rapid changes in NAMOC strength during the deglaciation.

Modeling the effects of snowpack on heterotrophic respiration across northern temperate and high latitude regions: Comparison with measurements of atmospheric carbon dioxide in high latitudes

USGS Publications Warehouse

McGuire, A.D.; Melillo, J.M.; Randerson, J.T.; Parton, W.J.; Heimann, Martin; Meier, R.A.; Clein, Joy S.; Kicklighter, D.W.; Sauf, W.

2000-01-01

Simulations by global terrestrial biogeochemical models (TBMs) consistently underestimate the concentration of atmospheric carbon dioxide (CO2) at high latitude monitoring stations during the nongrowing season. We hypothesized that heterotrophic respiration is underestimated during the nongrowing season primarily because TBMs do not generally consider the insulative effects of snowpack on soil temperature. To evaluate this hypothesis, we compared the performance of baseline and modified versions of three TBMs in simulating the seasonal cycle of atmospheric CO2 at high latitude CO2 monitoring stations; the modified version maintained soil temperature at 0 ??C when modeled snowpack was present. The three TBMs include the Carnegie-Ames-Stanford Approach (CASA), Century, and the Terrestrial Ecosystem Model (TEM). In comparison with the baseline simulation of each model, the snowpack simulations caused higher releases of CO2 between November and March and greater uptake of CO2 between June and August for latitudes north of 30??N. We coupled the monthly estimates of CO2 exchange, the seasonal carbon dioxide flux fields generated by the HAMOCC3 seasonal ocean carbon cycle model, and fossil fuel source fields derived from standard sources to the three-dimensional atmospheric transport model TM2 forced by observed winds to simulate the seasonal cycle of atmospheric CO2 at each of seven high latitude monitoring stations, in comparison to the CO2 concentrations simulated with the baseline fluxes of each TBM, concentrations simulated using the snowpack fluxes are generally in better agreement with observed concentrations between August and March at each of the monitoring stations. Thus, representation of the insulative effects of snowpack in TBMs generally improves simulation of atmospheric CO2 concentrations in high latitudes during both the late growing season and nongrowing season. These simulations highlight the global importance of biogeochemical processes during the nongrowing season in estimating carbon balance of ecosystems in northern high and temperate latitudes.

Investigation of Surface Flux Feedbacks for Coupled Atmosphere-Ocean Anomalies

NASA Technical Reports Server (NTRS)

Roberts, J. Brent; Robertson, Pete

2010-01-01

The use of "dynamical coupling" rules allows for identifying coupled vs. uncoupled anomalies and one-way interaction. Results of this study are consistent with those of Pena et al. (2003,2004) although using a more recent reanalysis at higher resolution. Find more atmosphere-forcing coupled anomalies in the extratropics and ocean-forcing anomalies in the tropics. The LHF and SWR show the largest magnitude anomalies in the composite analysis. The turbulent flux responses are due to interactions between the differing responses in wind speed and near-surface gradients. The radiative fluxes responses are primarily tied to changes in cloud fraction, as expected, though longwave response can be tied more to changes in the upwelling component.

WRF-Fire: coupled weather-wildland fire modeling with the weather research and forecasting model

Treesearch

Janice L. Coen; Marques Cameron; John Michalakes; Edward G. Patton; Philip J. Riggan; Kara M. Yedinak

2012-01-01

A wildland fire behavior module (WRF-Fire) was integrated into the Weather Research and Forecasting (WRF) public domain numerical weather prediction model. The fire module is a surface fire behavior model that is two-way coupled with the atmospheric model. Near-surface winds from the atmospheric model are interpolated to a finer fire grid and used, with fuel properties...

CERES FM6 Edition1-CV Product Release

Atmospheric Science Data Center

2018-06-13

... Wednesday, June 13, 2018 The Atmospheric Science Data Center (ASDC) at NASA Langley Research Center in collaboration with the CERES Science Team announces the release of the first Joint Polar Satellite System 1 ...

Geologic signatures of atmospheric effects on impact cratering on Venus

NASA Technical Reports Server (NTRS)

1996-01-01

Highlights of the research include geologic signatures of impact energy and atmospheric response to crater formation. Laboratory experiments were performed at the NASA Ames Vertical Gun Range (AVGR) to assess the interaction between disrupted impactor and atmosphere during entry, and to assess the energy coupling between impacts and the surrounding atmosphere. The Schlieren imaging at the AVGR was used in combination with Magellan imaging and theoretical studies to study the evolution of the impactor following impact. The Schlieren imaging documented the downrange blast front created by vaporization during oblique impacts. Laboratory experiments allowed assessing the effect of impact angle on coupling efficiency with an atmosphere. And the impact angle's effect on surface blasts and run-out flows allowed the distinction of crater clusters created by simultaneous impacts from those created by isolated regions of older age.

Sounding rocket/ground-based observation campaign to study Medium-Scale Traveling Ionospheric Disturbances (MSTID)

NASA Astrophysics Data System (ADS)

Yamamoto, Mamoru; Otsuka, Yuichi; Abe, Takumi; Yokoyama, Tatsuhiro; Bernhardt, Paul; Watanabe, Shigeto; Yamamoto, Masa-yuki; Larsen, Miguel; Saito, Akinori; Pfaff, Robert; Ishisaka, Keigo

2012-07-01

An observation campaign is under preparation. It is to launch sounding rockets S-520-27 and S-310-42 from Uchinoura Space Center of JAXA, while ground-based instruments measure waves in the ionosphere. The main purpose of the study is to reveal seeding mechanism of Medium-Scale Traveling Ionospheric Disturbances (MSTID). The MSTID is enhanced in the summer nighttime of the mid-latitude ionosphere. The MSTID is not only a simple reflection of atmospheric waves to the ionosphere, but includes complicated processes including the electromagnetic coupling of the F- and E-regions, and inter-hemisphere coupling of the ionosphere. We will measure ionospheric parameters such as electron density and electric fields together with neutral winds in the E- and F-regions. TMA and Lithium release experiment will be conducted with S-310-42 and S-520-27 rockets, respectively. The observation campaign is planned in summer 2012 or 2013. In the presentation we will overview characteristics of MSTID, and show plan and current status of the project. We also touch results from the sounding rocket S-520-26 that was launched on January 12, 2012. We will show results of the rocket-ground dual-band beacon experiment.

Antiapoptotic activity of argon and xenon

PubMed Central

Spaggiari, Sabrina; Kepp, Oliver; Rello-Varona, Santiago; Chaba, Kariman; Adjemian, Sandy; Pype, Jan; Galluzzi, Lorenzo; Lemaire, Marc; Kroemer, Guido

2013-01-01

Although chemically non-reactive, inert noble gases may influence multiple physiological and pathological processes via hitherto uncharacterized physical effects. Here we report a cell-based detection system for assessing the effects of pre-defined gas mixtures on the induction of apoptotic cell death. In this setting, the conventional atmosphere for cell culture was substituted with gas combinations, including the same amount of oxygen (20%) and carbon dioxide (5%) but 75% helium, neon, argon, krypton, or xenon instead of nitrogen. The replacement of nitrogen with noble gases per se had no effects on the viability of cultured human osteosarcoma cells in vitro. Conversely, argon and xenon (but not helium, neon, and krypton) significantly limited cell loss induced by the broad-spectrum tyrosine kinase inhibitor staurosporine, the DNA-damaging agent mitoxantrone and several mitochondrial toxins. Such cytoprotective effects were coupled to the maintenance of mitochondrial integrity, as demonstrated by means of a mitochondrial transmembrane potential-sensitive dye and by assessing the release of cytochrome c into the cytosol. In line with this notion, argon and xenon inhibited the apoptotic activation of caspase-3, as determined by immunofluorescence microscopy coupled to automated image analysis. The antiapoptotic activity of argon and xenon may explain their clinically relevant cytoprotective effects. PMID:23907115

View of ANDE release from orbiter Discovery payload bay

NASA Image and Video Library

2006-12-21

S116-E-07828 (21 Dec. 2006) --- As seen through windows on the aft flight deck of Space Shuttle Discovery, a Department of Defense pico-satellite known as Atmospheric Neutral Density Experiment (ANDE) is released from the shuttle's payload bay by STS-116 crewmembers. ANDE consists of two micro-satellites which will measure the density and composition of the low Earth orbit (LEO) atmosphere while being tracked from the ground. The data will be used to better predict the movement of objects in orbit.

Atmospheric release model for the E-area low-level waste facility: Updates and modifications

DOE Office of Scientific and Technical Information (OSTI.GOV)

None, None

The atmospheric release model (ARM) utilizes GoldSim® Monte Carlo simulation software (GTG, 2017) to evaluate the flux of gaseous radionuclides as they volatilize from E-Area disposal facility waste zones, diffuse into the air-filled soil pores surrounding the waste, and emanate at the land surface. This report documents the updates and modifications to the ARM for the next planned E-Area PA considering recommendations from the 2015 PA strategic planning team outlined by Butcher and Phifer.

Determination and impact of surface radiative processes for TOGA COARE

NASA Technical Reports Server (NTRS)

Curry, Judith A.; Ackerman, Thomas; Rossow, William B.; Webster, Peter J.

1991-01-01

Experiments using atmospheric general circulation models have shown that the atmospheric circulation is very sensitive to small changes in sea surface temperature in the tropical western Pacific Ocean warm pool region. The mutual sensitivity of the ocean and the atmosphere in the warm pool region places stringent requirements on models of the coupled ocean atmosphere system. At present, the situation is such that diagnostic studies using available data sets have been unable to balance the surface energy budget in the warm pool region to better than 50 to 80 W/sq m. The Tropical Ocean Global Atmosphere (TOGA) Coupled Ocean Atmosphere Response Experiment (COARE) is an observation and modelling program that aims specifically at the elucidation of the physical process which determine the mean and transient state of the warm pool region and the manner in which the warm pool interacts with the global ocean and atmosphere. This project focuses on one very important aspect of the ocean atmosphere interface component of TOGA COARE, namely the temporal and spatial variability of surface radiative fluxes in the warm pool region.

Modeling High-Resolution Coastal Ocean Dynamics with COAMPS: System Overview, Applications and Future Directions

NASA Astrophysics Data System (ADS)

Allard, R. A.; Campbell, T. J.; Edwards, K. L.; Smith, T.; Martin, P.; Hebert, D. A.; Rogers, W.; Dykes, J. D.; Jacobs, G. A.; Spence, P. L.; Bartels, B.

2014-12-01

The Coupled Ocean Atmosphere Mesoscale Prediction System (COAMPS®) is an atmosphere-ocean-wave modeling system developed by the Naval Research Laboratory which can be configured to cycle regional forecasts/analysis models in single-model (atmosphere, ocean, and wave) or coupled-model (atmosphere-ocean, ocean-wave, and atmosphere-ocean-wave) modes. The model coupling is performed using the Earth System Modeling Framework (ESMF). The ocean component is the Navy Coastal Ocean Model (NCOM), and the wave components include Simulating WAves Nearshore (SWAN) and WaveWatch-III. NCOM has been modified to include wetting and drying, the effects of Stokes drift current, wave radiation stresses due to horizontal gradients of the momentum flux of surface waves, enhancement of bottom drag in shallow water, and enhanced vertical mixing due to Langmuir turbulence. An overview of the modeling system including ocean data assimilation and specification of boundary conditions will be presented. Results from a high-resolution (10-250m) modeling study from the Surfzone Coastal Oil Pathways Experiment (SCOPE) near Ft. Walton Beach, Florida in December 2013 will be presented. ®COAMPS is a registered trademark of the Naval Research Laboratory

Development of a High-Resolution Climate Model for Future Climate Change Projection on the Earth Simulator

NASA Astrophysics Data System (ADS)

Kanzawa, H.; Emori, S.; Nishimura, T.; Suzuki, T.; Inoue, T.; Hasumi, H.; Saito, F.; Abe-Ouchi, A.; Kimoto, M.; Sumi, A.

2002-12-01

The fastest supercomputer of the world, the Earth Simulator (total peak performance 40TFLOPS) has recently been available for climate researches in Yokohama, Japan. We are planning to conduct a series of future climate change projection experiments on the Earth Simulator with a high-resolution coupled ocean-atmosphere climate model. The main scientific aims for the experiments are to investigate 1) the change in global ocean circulation with an eddy-permitting ocean model, 2) the regional details of the climate change including Asian monsoon rainfall pattern, tropical cyclones and so on, and 3) the change in natural climate variability with a high-resolution model of the coupled ocean-atmosphere system. To meet these aims, an atmospheric GCM, CCSR/NIES AGCM, with T106(~1.1o) horizontal resolution and 56 vertical layers is to be coupled with an oceanic GCM, COCO, with ~ 0.28ox 0.19o horizontal resolution and 48 vertical layers. This coupled ocean-atmosphere climate model, named MIROC, also includes a land-surface model, a dynamic-thermodynamic seaice model, and a river routing model. The poles of the oceanic model grid system are rotated from the geographic poles so that they are placed in Greenland and Antarctic land masses to avoild the singularity of the grid system. Each of the atmospheric and the oceanic parts of the model is parallelized with the Message Passing Interface (MPI) technique. The coupling of the two is to be done with a Multi Program Multi Data (MPMD) fashion. A 100-model-year integration will be possible in one actual month with 720 vector processors (which is only 14% of the full resources of the Earth Simulator).

Predictability of North Atlantic Multidecadal Climate Variability

PubMed

Griffies; Bryan

1997-01-10

Atmospheric weather systems become unpredictable beyond a few weeks, but climate variations can be predictable over much longer periods because of the coupling of the ocean and atmosphere. With the use of a global coupled ocean-atmosphere model, it is shown that the North Atlantic may have climatic predictability on the order of a decade or longer. These results suggest that variations of the dominant multidecadal sea surface temperature patterns in the North Atlantic, which have been associated with changes in climate over Eurasia, can be predicted if an adequate and sustainable system for monitoring the Atlantic Ocean exists.

The Torque of the Planet: NASA Researcher Uses NCCS Computers to Probe Atmosphere-Land-Ocean Coupling

NASA Technical Reports Server (NTRS)

2002-01-01

The study of Earth science is like a giant puzzle, says Braulio Sanchez. "The more you know about the individual pieces, the easier it is to fit them together." A researcher with Goddard's Space Geodesy Branch, Sanchez has been using NCCS supercomputer and mass storage resources to show how the angular momenta of the atmosphere, the oceans, and the solid Earth are dynamically coupled. Sanchez has calculated the magnitude of atmospheric torque on the planet and has determined some of the possible effects that torque has on Earth's rotation.

Behaviour of oceanic 137Cs following the Fukushima Daiichi Nuclear Power Plant accident for four years simulated numerically by a regional ocean model

NASA Astrophysics Data System (ADS)

Tsumune, D.; Tsubono, T.; Aoyama, M.; Misumi, K.; Tateda, Y.

2015-12-01

A series of accidents at the Fukushima Dai-ichi Nuclear Power Plant (1F NPP) following the earthquake and tsunami of 11 March 2011 resulted in the release of radioactive materials to the ocean by two major pathways, direct release from the accident site and atmospheric deposition.We reconstructed spatiotemporal variability of 137Cs activity in the regional ocean for four years by numerical model, such as a regional scale and the North Pacific scale oceanic dispersion models, an atmospheric transport model, a sediment transport model, a dynamic biological compartment model for marine biota and river runoff model. Direct release rate of 137Cs were estimated for four years after the accident by comparing simulated results and observed activities very close to the site. The estimated total amounts of directly release was 3.6±0.7 PBq. Directly release rate of 137Cs decreased exponentially with time by the end of December 2012 and then, was almost constant. Decrease rate were quite small after 2013. The daily release rate of 137Cs was estimated to be the order of magnitude of 1010 Bq/day by the end of March 2015. The activity of directly released 137Cs was detectable only in the coastal zone after December 2012. Simulated 137Cs activities attributable to direct release were in good agreement with observed activities, a result that implies the estimated direct release rate was reasonable. There is no observed data of 137Cs activity in the ocean from 11 to 21 March 2011. Observed data of marine biota should reflect the history of 137Cs activity in this early period. We reconstructed the history of 137Cs activity in this early period by considering atmospheric deposition, river input, rain water runoff from the 1F NPP site. The comparisons between simulated 137Cs activity of marine biota by a dynamic biological compartment and observed data also suggest that simulated 137Cs activity attributable to atmospheric deposition was underestimated in this early period. The simulated river flux of 137Cs to the ocean did not effect on 137Cs activity in the ocean even if the parameters in this simulation have uncertainties because of the lack of observed data in rivers in the earlier period.

Behaviour of oceanic 137Cs following the Fukushima Daiichi Nuclear Power Plant accident for four years simulated numerically by a regional ocean model

NASA Astrophysics Data System (ADS)

Torn, M. S.; Koven, C. D.; Riley, W. J.; Zhu, B.; Hicks Pries, C.; Phillips, C. L.

2014-12-01

A series of accidents at the Fukushima Dai-ichi Nuclear Power Plant (1F NPP) following the earthquake and tsunami of 11 March 2011 resulted in the release of radioactive materials to the ocean by two major pathways, direct release from the accident site and atmospheric deposition.We reconstructed spatiotemporal variability of 137Cs activity in the regional ocean for four years by numerical model, such as a regional scale and the North Pacific scale oceanic dispersion models, an atmospheric transport model, a sediment transport model, a dynamic biological compartment model for marine biota and river runoff model. Direct release rate of 137Cs were estimated for four years after the accident by comparing simulated results and observed activities very close to the site. The estimated total amounts of directly release was 3.6±0.7 PBq. Directly release rate of 137Cs decreased exponentially with time by the end of December 2012 and then, was almost constant. Decrease rate were quite small after 2013. The daily release rate of 137Cs was estimated to be the order of magnitude of 1010 Bq/day by the end of March 2015. The activity of directly released 137Cs was detectable only in the coastal zone after December 2012. Simulated 137Cs activities attributable to direct release were in good agreement with observed activities, a result that implies the estimated direct release rate was reasonable. There is no observed data of 137Cs activity in the ocean from 11 to 21 March 2011. Observed data of marine biota should reflect the history of 137Cs activity in this early period. We reconstructed the history of 137Cs activity in this early period by considering atmospheric deposition, river input, rain water runoff from the 1F NPP site. The comparisons between simulated 137Cs activity of marine biota by a dynamic biological compartment and observed data also suggest that simulated 137Cs activity attributable to atmospheric deposition was underestimated in this early period. The simulated river flux of 137Cs to the ocean did not effect on 137Cs activity in the ocean even if the parameters in this simulation have uncertainties because of the lack of observed data in rivers in the earlier period.

A simple analytical method for determining the atmospheric dispersion of upward-directed high velocity releases

NASA Astrophysics Data System (ADS)

Palazzi, E.

The evaluation of atmospheric dispersion of a cloud, arising from a sudden release of flammable or toxic materials, is an essential tool for properly designing flares, vents and other safety devices and to quantify the potential risk related to the existing ones or arising from the various kinds of accidents which can occur in chemical plants. Among the methods developed to treat the important case of upward-directed jets, Hoehne's procedure for determining the behaviour and extent of flammability zone is extensively utilized, particularly concerning petrochemical plants. In a previous study, a substantial simplification of the aforesaid procedure was achieved, by correlating the experimental data with an empirical formula, allowing to obtain a mathematical description of the boundaries of the flammable cloud. Following a theoretical approach, a most general model is developed in the present work, applicable to the various kinds of design problems and/or risk evaluation regarding upward-directed releases from high velocity sources. It is also demonstrated that the model gives conservative results, if applied outside the range of the Hoehne's experimental conditions. Moreover, with simple modifications, the same approach could be easily applied to deal with the atmospheric dispersion of anyhow directed releases.

Regional climatic effects of atmospheric SO2 on Mars

NASA Technical Reports Server (NTRS)

Postawko, S. E.; Fanale, F. P.

1992-01-01

The conditions under which the valley networks on Mars may have formed remains controversial. The magnitude of an atmospheric greenhouse effect by an early massive CO2 atmosphere has recently been questioned by Kasting. Recent calculations indicate that if solar luminosity were less than about 86 percent of its current value, formation of CO2 clouds in the Martian atmosphere would depress the atmospheric lapse rate and reduce the magnitude of surface warming. In light of recent revisions of magma generation on Mars during each Martian epoch, and the suggestions by Wanke et al. that the role of liquid SO2 should be more carefully explored, we have recalculated the potential greenhouse warming by atmospheric SO2 on Mars, with an emphasis on more localized effects. In the vicinity of an active eruption, the concentration of atmospheric SO2 will be higher than if it is assumed that the erupted SO2 is instantaneously globally distributed. The local steady-state concentration of SO2 is a function of the rate at which it is released, its atmospheric lifetime, and the rate at which local winds act to disperse the SO2. We have made estimates of eruption rates, length of eruption, and dispersion rates of volcanically released SO2, for a variety of atmospheric conditions and atmospheric lifetimes of SO2 to explore the maximum regional climatic effect of SO2.

3D modeling of lightning-induced electromagnetic pulses on Venus, Jupiter and Saturn

NASA Astrophysics Data System (ADS)

Pérez-Invernón, Francisco J.; Luque, Alejandro; Gordillo-Vázquez, Francisco J.

2017-04-01

Atmospheric electricity is a common phenomenon in some planets of The Solar System. We know that atmospheric discharges exist on Earth and gaseous planets; however, some characteristics of lightning on Saturn and Jupiter as well as their relevance on the effects of lightning in the atmospheres of these planets are still unknown. In the case of Venus, there exist some radio evidences of lightning, but the lack of optical observations suggests exploring indirect methods of detection, such as searching for lightning-induced transient optical emissions from the upper atmosphere. The Akatsuki probe, currently orbiting Venus, is equipped with a camera whose temporal resolution is high enough to detect optical emissions from lightning discharges and to measure nightglow enhancements. In this work, we extend previous models [1,2] to investigate the chemical impact and transient optical emissions produced by possible lightning-emitted electromagnetic pulses (EMP) in Venus, Saturn and Jupiter. Using a 3D FDTD ("Finite Differences Time Domain") model we solve the Maxwell equations coupled with the Langevin equation for electrons [3] and with a kinetic scheme, different for each planetary atmosphere. This method is useful to investigate the temporal and spatial impact of lightning-induced electromagnetic fields in the atmosphere of each planet for different lightning characteristics (e.g. energy released, orientation). This 3D FDTD model allows us to include the saturnian and jovian background magnetic field inclination and magnitude at different latitudes, and to determine the effects of different lightning channel inclinations. Results provide useful information to interpret lightning observations on giant gaseous planets and in the search for indirect optical signals from atmospheric discharge on Venus such as fast nightglow transient enhancements related to lightning as seen on Earth. Furthermore, we underline the observation of electrical discharges characteristics as a powerful tool to obtain information about planetary atmospheres, such as density profiles of electrons or other components. Our model may also be useful to extend some studies about the chemical impact of EMP pulses in the terrestrial atmosphere [4]. References [1] Luque, A., D. Dubrovin, F. J. Gordillo-Vázquez, U. Ebert, F. C. Parra-Rojas, Y. Yair, and C. Price (2014), Coupling between atmospheric layers in gaseous giant planets due to lightning-generated electromagnetic pulses, J. Geophys. Res. (Space Phys), 119, 8705, doi: 10.1002/2014JA020457. [2] Pérez-Invernón, F. J., A. Luque, and F. J. Gordillo-Vázquez (2016), Mesospheric optical signatures of possible lightning on Venus, J. Geophys. Res. (Space Phys), 121, 7026, doi: 10.1029/2016JA022886. [3] Lee, J. H., and D. K. Kalluri (1999), Three-dimensional FDTD simulation of electromagnetic wave transformation in a dynamic inhomogeneous magnetized plasma, IEEE Transactions on Antennas and Propagation, 47, 1146, doi:10.1109/8.785745. [4] Marshall, R. A., U. S. Inan, and V. S. Glukhov (2010), Elves and associated electron density changes due to cloud-to-ground and in-cloud lightning discharges, J. Geophys. Res. (Space Phys), 115, A00E17, doi:10.1029/2009JA014469.

Corrective Action Decision Document/Corrective Action Plan for Corrective Action Unit 104: Area 7 Yucca Flat Atmospheric Test Sites Nevada National Security Site, Nevada, Revision 0

DOE Office of Scientific and Technical Information (OSTI.GOV)

Patrick Matthews

2012-10-01

CAU 104 comprises the following corrective action sites (CASs): • 07-23-03, Atmospheric Test Site T-7C • 07-23-04, Atmospheric Test Site T7-1 • 07-23-05, Atmospheric Test Site • 07-23-06, Atmospheric Test Site T7-5a • 07-23-07, Atmospheric Test Site - Dog (T-S) • 07-23-08, Atmospheric Test Site - Baker (T-S) • 07-23-09, Atmospheric Test Site - Charlie (T-S) • 07-23-10, Atmospheric Test Site - Dixie • 07-23-11, Atmospheric Test Site - Dixie • 07-23-12, Atmospheric Test Site - Charlie (Bus) • 07-23-13, Atmospheric Test Site - Baker (Buster) • 07-23-14, Atmospheric Test Site - Ruth • 07-23-15, Atmospheric Test Site T7-4 •more » 07-23-16, Atmospheric Test Site B7-b • 07-23-17, Atmospheric Test Site - Climax These 15 CASs include releases from 30 atmospheric tests conducted in the approximately 1 square mile of CAU 104. Because releases associated with the CASs included in this CAU overlap and are not separate and distinguishable, these CASs are addressed jointly at the CAU level. The purpose of this CADD/CAP is to evaluate potential corrective action alternatives (CAAs), provide the rationale for the selection of recommended CAAs, and provide the plan for implementation of the recommended CAA for CAU 104. Corrective action investigation (CAI) activities were performed from October 4, 2011, through May 3, 2012, as set forth in the CAU 104 Corrective Action Investigation Plan.« less

Methodology for prediction and estimation of consequences of possible atmospheric releases of hazardous matter: "Kursk" submarine study

NASA Astrophysics Data System (ADS)

Baklanov, A.; Mahura, A.; Sørensen, J. H.

2003-06-01

There are objects with some periods of higher than normal levels of risk of accidental atmospheric releases (nuclear, chemical, biological, etc.). Such accidents or events may occur due to natural hazards, human errors, terror acts, and during transportation of waste or various operations at high risk. A methodology for risk assessment is suggested and it includes two approaches: 1) probabilistic analysis of possible atmospheric transport patterns using long-term trajectory and dispersion modelling, and 2) forecast and evaluation of possible contamination and consequences for the environment and population using operational dispersion modelling. The first approach could be applied during the preparation stage, and the second - during the operation stage. The suggested methodology is applied on an example of the most important phases (lifting, transportation, and decommissioning) of the ``Kursk" nuclear submarine operation. It is found that the temporal variability of several probabilistic indicators (fast transport probability fields, maximum reaching distance, maximum possible impact zone, and average integral concentration of 137Cs) showed that the fall of 2001 was the most appropriate time for the beginning of the operation. These indicators allowed to identify the hypothetically impacted geographical regions and territories. In cases of atmospheric transport toward the most populated areas, the forecasts of possible consequences during phases of the high and medium potential risk levels based on a unit hypothetical release (e.g. 1 Bq) are performed. The analysis showed that the possible deposition fractions of 10-11 (Bq/m2) over the Kola Peninsula, and 10-12 - 10-13 (Bq/m2) for the remote areas of the Scandinavia and Northwest Russia could be observed. The suggested methodology may be used successfully for any potentially dangerous object involving risk of atmospheric release of hazardous materials of nuclear, chemical or biological nature.

Methodology for prediction and estimation of consequences of possible atmospheric releases of hazardous matter: "Kursk"? submarine study

NASA Astrophysics Data System (ADS)

Baklanov, A.; Mahura, A.; Sørensen, J. H.

2003-03-01

There are objects with some periods of higher than normal levels of risk of accidental atmospheric releases (nuclear, chemical, biological, etc.). Such accidents or events may occur due to natural hazards, human errors, terror acts, and during transportation of waste or various operations at high risk. A methodology for risk assessment is suggested and it includes two approaches: 1) probabilistic analysis of possible atmospheric transport patterns using long-term trajectory and dispersion modelling, and 2) forecast and evaluation of possible contamination and consequences for the environment and population using operational dispersion modelling. The first approach could be applied during the preparation stage, and the second - during the operation stage. The suggested methodology is applied on an example of the most important phases (lifting, transportation, and decommissioning) of the "Kursk" nuclear submarine operation. It is found that the temporal variability of several probabilistic indicators (fast transport probability fields, maximum reaching distance, maximum possible impact zone, and average integral concentration of 137Cs) showed that the fall of 2001 was the most appropriate time for the beginning of the operation. These indicators allowed to identify the hypothetically impacted geographical regions and territories. In cases of atmospheric transport toward the most populated areas, the forecasts of possible consequences during phases of the high and medium potential risk levels based on a unit hypothetical release are performed. The analysis showed that the possible deposition fractions of 1011 over the Kola Peninsula, and 10-12 - 10-13 for the remote areas of the Scandinavia and Northwest Russia could be observed. The suggested methodology may be used successfully for any potentially dangerous object involving risk of atmospheric release of hazardous materials of nuclear, chemical or biological nature.

Terrestrial and Martian weathering signatures of xenon components in shergottite mineral separates

NASA Astrophysics Data System (ADS)

Cartwright, J. A.; Ocker, K. D.; Crowther, S. A.; Burgess, R.; Gilmour, J. D.

2010-08-01

Xenon-isotopic ratios, step-heating release patterns, and gas concentrations of mineral separates from Martian shergottites Roberts Massif (RBT) 04262, Dar al Gani (DaG) 489, Shergotty, and Elephant Moraine (EET) 79001 lithology B are reported. Concentrations of Martian atmospheric xenon are similar in mineral separates from all meteorites, but more weathered samples contain more terrestrial atmospheric xenon. The distributions of xenon from the Martian and terrestrial atmospheres among minerals in any one sample are similar, suggesting similarities in the processes by which they were acquired. However, in opaque and maskelynite fractions, Martian atmospheric xenon is released at higher temperatures than terrestrial atmospheric xenon. It is suggested that both Martian and terrestrial atmospheric xenon were initially introduced by weathering (low temperature alteration processes). However, the Martian component was redistributed by shock, accounting for its current residence in more retentive sites. The presence or absence of detectable 129Xe from the Martian atmosphere in mafic minerals may correspond to the extent of crustal contamination of the rock's parent melt. Variable contents of excess 129Xe contrast with previously reported consistent concentrations of excess 40Ar, suggesting distinct sources contributed these gases to the parent magma.

Emission profiles of polychlorinated dibenzodioxins, polychlorinated dibenzofurans (PCDD/Fs), dioxin-like PCBs and hexachlorobenzene (HCB) from secondary metallurgy industries in Portugal.

PubMed

Antunes, Pedro; Viana, Paula; Vinhas, Tereza; Rivera, J; Gaspar, Elvira M S M

2012-09-01

This paper reports, for the first time, a study of dioxin emissions from 10 siderurgies and metallurgies, secondary copper, aluminum and lead metallurgies, in Portugal. The study reports the emission factors and total emission amounts of PCDD/Fs, dioxin-like PCBs and hexachlorobenzene (HCB). The congener patterns were characterized and are discussed. The results showed that the total amount of PCDFs is higher than PCDDs in flue gas of each industrial unit. The toxic equivalent emission factors of pollutants emitted are 3098-3338 ngI-TEQt(-1) for PCDD/Fs and 597-659 ng I-TEQt(-1) for dioxin-like PCBs in siderurgies production (total estimated emission amounts released to atmosphere of 3.9-4.5 g I-TEQyr(-1)), 50-152 ng I-TEQt(-1) for PCDD/Fs and 24-121 ng I-TEQt(-1) for dioxin-like PCBs in ferrous foundries production (total estimated emission amounts released to atmosphere of 0.0010-0.0016 g I-TEQyr(-1)) and 5.8-5715 ng I-TEQt(-1) for PCDD/Fs and 0.49-259 ng I-TEQt(-1) for dioxin-like PCBs in non-ferrous foundries production (total estimated emission amounts released to atmosphere of 0.00014-0.12 g I-TEQyr(-1)). The HCB emission from siderurgies production is 0.94-3.2 mg t(-1) (total estimated emission amounts released 0.94-3.8 g yr(-1)), being much smaller, residual, in the emissions of the other types of plants (0.0012-0.026 mg t(-1) production and total estimated emission amounts released to atmosphere of 0.013-1.7 mg yr(-1)). Copyright © 2012 Elsevier Ltd. All rights reserved.

First estimates of the contribution of CaCO3 precipitation to the release of CO2 to the atmosphere during young sea ice growth

NASA Astrophysics Data System (ADS)

Geilfus, N.-X.; Carnat, G.; Dieckmann, G. S.; Halden, N.; Nehrke, G.; Papakyriakou, T.; Tison, J.-L.; Delille, B.

2013-01-01

report measurements of pH, total alkalinity, air-ice CO2 fluxes (chamber method), and CaCO3 content of frost flowers (FF) and thin landfast sea ice. As the temperature decreases, concentration of solutes in the brine skim increases. Along this gradual concentration process, some salts reach their solubility threshold and start precipitating. The precipitation of ikaite (CaCO3.6H2O) was confirmed in the FF and throughout the ice by Raman spectroscopy and X-ray analysis. The amount of ikaite precipitated was estimated to be 25 µmol kg-1 melted FF, in the FF and is shown to decrease from 19 to 15 µmol kg-1 melted ice in the upper part and at the bottom of the ice, respectively. CO2 release due to precipitation of CaCO3 is estimated to be 50 µmol kg-1 melted samples. The dissolved inorganic carbon (DIC) normalized to a salinity of 10 exhibits significant depletion in the upper layer of the ice and in the FF. This DIC loss is estimated to be 2069 µmol kg-1 melted sample and corresponds to a CO2 release from the ice to the atmosphere ranging from 20 to 40 mmol m-2 d-1. This estimate is consistent with flux measurements of air-ice CO2 exchange. Our measurements confirm previous laboratory findings that growing young sea ice acts as a source of CO2 to the atmosphere. CaCO3 precipitation during early ice growth appears to promote the release of CO2 to the atmosphere; however, its contribution to the overall release by newly formed ice is most likely minor.

Anthropogenic 129I in the atmosphere: overview over major sources, transport processes and deposition pattern.

PubMed

Reithmeier, H; Lazarev, V; Rühm, W; Nolte, E

2010-10-01

Wet and, to a lesser extent, dry deposition of atmospheric (129)I are known to represent the dominating processes responsible for (129)I in continental environmental samples that are remote from (129)I sources and not directly influenced by any liquid (129)I release of nuclear installations. Up to now, however, little is known about the major emitters and the related global deposition pattern of (129)I. In this work an overview over major sources of (129)I is given, and hitherto unknown time-dependent releases from these were estimated. Total gaseous (129)I releases from the US and former Soviet reprocessing facilities Hanford, Savannah River, Mayak, Seversk and Zheleznogorsk were found to have been 0.53, 0.27, 1.05, 0.23 and 0.14TBq, respectively. These facilities were thus identified as major airborne (129)I emitters. The global deposition pattern due to the (129)I released, depending on geographic latitude and longitude, and on time was studied using a box model describing the global atmospheric transport and deposition of (129)I. The model predictions are compared to (129)I concentrations measured by means of Accelerator Mass Spectrometry (AMS) in water samples that were collected from various lakes in Asia, Africa, America and New Zealand, and to published values. As a result, both pattern and temporal evolution of (129)I deposition values measured in and calculated for different types of environmental samples are, in general, in good agreement. This supports our estimate on atmospheric (129)I releases and the considered substantial transport and deposition mechanisms in our model calculations. Copyright 2010 Elsevier B.V. All rights reserved.

Isotopic signature of atmospheric xenon released from light water reactors.

PubMed

Kalinowski, Martin B; Pistner, Christoph

2006-01-01

A global monitoring system for atmospheric xenon radioactivity is being established as part of the International Monitoring System to verify compliance with the Comprehensive Nuclear-Test-Ban Treaty (CTBT). The isotopic activity ratios of (135)Xe, (133m)Xe, (133)Xe and (131m)Xe are of interest for distinguishing nuclear explosion sources from civilian releases. Simulations of light water reactor (LWR) fuel burn-up through three operational reactor power cycles are conducted to explore the possible xenon isotopic signature of nuclear reactor releases under different operational conditions. It is studied how ratio changes are related to various parameters including the neutron flux, uranium enrichment and fuel burn-up. Further, the impact of diffusion and mixing on the isotopic activity ratio variability are explored. The simulations are validated with reported reactor emissions. In addition, activity ratios are calculated for xenon isotopes released from nuclear explosions and these are compared to the reactor ratios in order to determine whether the discrimination of explosion releases from reactor effluents is possible based on isotopic activity ratios.

A Review of Low Frequency Electromagnetic Wave Phenomena Related to Tropospheric-Ionospheric Coupling Mechanisms

NASA Technical Reports Server (NTRS)

Simoes, Fernando; Pfaff, Robert; Berthelier, Jean-Jacques; Klenzing, Jeffrey

2012-01-01

Investigation of coupling mechanisms between the troposphere and the ionosphere requires a multidisciplinary approach involving several branches of atmospheric sciences, from meteorology, atmospheric chemistry, and fulminology to aeronomy, plasma physics, and space weather. In this work, we review low frequency electromagnetic wave propagation in the Earth-ionosphere cavity from a troposphere-ionosphere coupling perspective. We discuss electromagnetic wave generation, propagation, and resonance phenomena, considering atmospheric, ionospheric and magnetospheric sources, from lightning and transient luminous events at low altitude to Alfven waves and particle precipitation related to solar and magnetospheric processes. We review in situ ionospheric processes as well as surface and space weather phenomena that drive troposphere-ionosphere dynamics. Effects of aerosols, water vapor distribution, thermodynamic parameters, and cloud charge separation and electrification processes on atmospheric electricity and electromagnetic waves are reviewed. We also briefly revisit ionospheric irregularities such as spread-F and explosive spread-F, sporadic-E, traveling ionospheric disturbances, Trimpi effect, and hiss and plasma turbulence. Regarding the role of the lower boundary of the cavity, we review transient surface phenomena, including seismic activity, earthquakes, volcanic processes and dust electrification. The role of surface and atmospheric gravity waves in ionospheric dynamics is also briefly addressed. We summarize analytical and numerical tools and techniques to model low frequency electromagnetic wave propagation and solving inverse problems and summarize in a final section a few challenging subjects that are important for a better understanding of tropospheric-ionospheric coupling mechanisms.

Regional Responses to Black Carbon Aerosols: The Importance of Air-Sea Interaction

NASA Astrophysics Data System (ADS)

Gnanadesikan, A.; Scott, A. A.; Pradal, M.-A.; Seviour, W. J. M.; Waugh, D. W.

2017-12-01

The impact of modern black carbon aerosols on climate via their changes in radiative balance is studied using a coupled model where sea surface temperatures (SSTs) are allowed to vary and an atmosphere-only version of the same model where SSTs are held fixed. Allowing the ocean to respond is shown to have a profound impact on the pattern of temperature change. Particularly, large impacts are found in the North Pacific (which cools by up to 1 K in the coupled model) and in north central Asia (which warms in the coupled simulation and cools in the fixed SST simulation). Neither set of experiments shows large changes in surface temperatures in the Southeast Asian region where the atmospheric burden of black carbon is highest. These results are related to the stabilization of the atmosphere and changes in oceanic heat transport. Over the North Pacific, atmospheric stabilization results in an increase in stratiform clouds. The resulting shading reduces evaporation, freshening the surface layer of the ocean and reducing the inflow of warm subtropical waters. Over the land, a delicate balance between greater atmospheric absorption, shading of the surface and changes in latent cooling of the surface helps to determine whether warming or cooling is seen. Our results emphasize the importance of coupling in determining the response of the climate system to black carbon and suggest that black carbon may play an important role in modulating climate change over the North Pacific.

Regional Effects of the Mount Pinatubo Eruption on the Middle East and the Red Sea

NASA Astrophysics Data System (ADS)

Osipov, Sergey; Stenchikov, Georgiy

2017-11-01

The 1991 eruption of Mount Pinatubo had dramatic effects on the regional climate in the Middle East. Though acknowledged, these effects have not been thoroughly studied. To fill this gap and to advance understanding of the mechanisms that control variability in the Middle East's regional climate, we simulated the impact of the 1991 Pinatubo eruption using a regional coupled ocean-atmosphere modeling system set for the Middle East and North Africa (MENA) domain. We used the Coupled Ocean-Atmosphere-Wave-Sediment Transport (COAWST) framework, which couples the Weather Research and Forecasting Model (WRF) model with the Regional Oceanic Modeling System (ROMS). We modified the WRF model to account for the radiative effect of volcanic aerosols. Our coupled ocean-atmosphere simulations verified by available observations revealed strong perturbations in the energy balance of the Red Sea, which drove thermal and circulation responses. Our modeling approach allowed us to separate changes in the atmospheric circulation caused by the impact of the volcano from direct regional radiative cooling from volcanic aerosols. The atmospheric circulation effect was significantly stronger than the direct volcanic aerosols effect. We found that the Red Sea response to the Pinatubo eruption was stronger and qualitatively different from that of the global ocean system. Our results suggest that major volcanic eruptions significantly affect the climate in the Middle East and the Red Sea and should be carefully taken into account in assessments of long-term climate variability and warming trends in MENA and the Red Sea.

Arabidopsis seed production limited by CO2 in simulated space experiments

NASA Technical Reports Server (NTRS)

Hoshizaki, T.

1984-01-01

Several generations of Arabidopsis thaliana were grown axenically from seed to seed on nutrient agar medium. The Arabidopsis plants produce seeds within 30 days after seeding, when grown either in containers open to the ambient atmosphere or in large sealed jars, but not in sealed test tubes. Moreover, the plant height was directly proportional to the size of the sealed container. Periodic analyses of the CO2 levels in the sealed containers has shown a decrease during the first week, but a tenfold increase in the following weeks. It is speculated that, by the end of the second week, the cotyledons entering the senescence stage would release ethylene into the culture atmosphere with a concomitant release of CO2, which in turn would induce further release of ethylene, hastening the senescence process in other tissues. Thus, in a controlled ecological life-support system of a space station, various components of the plant atmosphere may have to be maintained within the prescribed limits.

Atmospheric contribution of gas emissions from Augustine volcano, Alaska during the 2006 eruption

USGS Publications Warehouse

McGee, K.A.; Doukas, M.P.; McGimsey, R.G.; Neal, C.A.; Wessels, R.L.

2008-01-01

Airborne surveillance of gas emissions from Augustine for SO2, CO2 and H2S showed no evidence of anomalous degassing from 1990 through May 2005. By December 20, 2005, Augustine was degassing 660 td-1 of SO2, and ten times that by January 4, 2006. The highest SO2 emission rate measured during the 2006 eruption was 8650 td-1 (March 1); for CO2, 13000 td-1 (March 9), and H2S, 8 td-1 (January 19). Thirty-four SO2 measurements were made from December 2005 through 2006, with 9 each for CO2 and H2S. Augustine released 1 ?? 106 tonnes of CO2 to the atmosphere during 2006, a level similar to the output of a medium-sized natural gas-fired power plant, and thus was not a significant contributor of greenhouse gas to the atmosphere compared to anthropogenic sources. Augustine released about 5 ?? 105 tonnes of SO2 during 2006, similar to that released in 1976 and 1986.

Analytical Model for Diffusive Evaporation of Sessile Droplets Coupled with Interfacial Cooling Effect.

PubMed

Nguyen, Tuan A H; Biggs, Simon R; Nguyen, Anh V

2018-05-30

Current analytical models for sessile droplet evaporation do not consider the nonuniform temperature field within the droplet and can overpredict the evaporation by 20%. This deviation can be attributed to a significant temperature drop due to the release of the latent heat of evaporation along the air-liquid interface. We report, for the first time, an analytical solution of the sessile droplet evaporation coupled with this interfacial cooling effect. The two-way coupling model of the quasi-steady thermal diffusion within the droplet and the quasi-steady diffusion-controlled droplet evaporation is conveniently solved in the toroidal coordinate system by applying the method of separation of variables. Our new analytical model for the coupled vapor concentration and temperature fields is in the closed form and is applicable for a full range of spherical-cap shape droplets of different contact angles and types of fluids. Our analytical results are uniquely quantified by a dimensionless evaporative cooling number E o whose magnitude is determined only by the thermophysical properties of the liquid and the atmosphere. Accordingly, the larger the magnitude of E o , the more significant the effect of the evaporative cooling, which results in stronger suppression on the evaporation rate. The classical isothermal model is recovered if the temperature gradient along the air-liquid interface is negligible ( E o = 0). For substrates with very high thermal conductivities (isothermal substrates), our analytical model predicts a reversal of temperature gradient along the droplet-free surface at a contact angle of 119°. Our findings pose interesting challenges but also guidance for experimental investigations.

The Impact of Land-Atmosphere Coupling on the 2017 Northern Great Plains Drought

NASA Astrophysics Data System (ADS)

Roundy, J. K.; Santanello, J. A., Jr.

2017-12-01

In a changing climate, the potential for increased frequency and duration of drought implies devastating impacts on many aspects of society. The negative impacts of drought can be reduced through informing sustainable water management made possible by real-time monitoring and prediction. The refinement of forecast models is best realized through large-scale observation based datasets, yet there are few of these datasets currently available. The Coupling Drought Index (CDI) is a metric based on the persistence of Land-Atmosphere (L-A) coupling into distinct regimes derived from observations of the land and atmospheric state. The coupling regime persistence has been shown to relate to drought intensification and recovery and is the basis for the Coupling Statistical Model (CSM), which uses a Markov Chain framework to make statistical predictions. The CDI and CSM have been used to understand the predictability of L-A interactions in NCEP's Climate Forecasts System version 2 (CFSv2) and indicated that the forecasts exhibit strong biases in the L-A coupling that produced biases in the precipitation and limited the predictability of drought. The CDI can also be derived exclusively from satellite data which provides an observational large-scale metric of L-A coupling and drought evolution. This provides a unique observational tool for understanding the persistence and intensification of drought through land-atmosphere interactions. During the Spring and Summer of 2017, a drought developed over the Norther great plains that caused substantial agricultural losses in parts of Montana and North and South Dakota. In this work, we use satellite derived CDI to explore the impact of Land-Atmosphere Interactions on the persistence and intensification of the 2017 Northern Great Plains drought. To do this we analyze and quantify the change in CDI at various spatial and temporal scales and correlate these changes with other drought indicators including the U.S. Drought Monitor (http://droughtmonitor.unl.edu). The 2017 Northern Great Plains drought is compared to previous droughts in the region and the predictability of 2017 drought from the CSM as well as future droughts for the area is assessed.

Methane Seepage on Mars: Where to Look and Why

NASA Astrophysics Data System (ADS)

Oehler, Dorothy Z.; Etiope, Giuseppe

2017-12-01

Methane on Mars is a topic of special interest because of its potential association with microbial life. The variable detections of methane by the Curiosity rover, orbiters, and terrestrial telescopes, coupled with methane's short lifetime in the martian atmosphere, may imply an active gas source in the planet's subsurface, with migration and surface emission processes similar to those known on Earth as "gas seepage." Here, we review the variety of subsurface processes that could result in methane seepage on Mars. Such methane could originate from abiotic chemical reactions, thermogenic alteration of abiotic or biotic organic matter, and ancient or extant microbial metabolism. These processes can occur over a wide range of temperatures, in both sedimentary and igneous rocks, and together they enhance the possibility that significant amounts of methane could have formed on early Mars. Methane seepage to the surface would occur preferentially along faults and fractures, through focused macro-seeps and/or diffuse microseepage exhalations. Our work highlights the types of features on Mars that could be associated with methane release, including mud-volcano-like mounds in Acidalia or Utopia; proposed ancient springs in Gusev Crater, Arabia Terra, and Valles Marineris; and rims of large impact craters. These could have been locations of past macro-seeps and may still emit methane today. Microseepage could occur through faults along the dichotomy or fractures such as those at Nili Fossae, Cerberus Fossae, the Argyre impact, and those produced in serpentinized rocks. Martian microseepage would be extremely difficult to detect remotely yet could constitute a significant gas source. We emphasize that the most definitive detection of methane seepage from different release candidates would be best provided by measurements performed in the ground or at the ground-atmosphere interface by landers or rovers and that the technology for such detection is currently available.

WARRP Decon-13: Subject Matter Expert (SME) Meeting Waste Screening and Waste Minimization Methodologies Project

DTIC Science & Technology

2012-08-01

radioactive material compares to Chernobyl . In looking at atmospheric releases of Cs- 137, there seems to be agreement that Fukushima releases were about 10...to 20% of those produced by the Chernobyl event. However, the Fukushima event has resulted in significant releases of contaminated water to the...ocean. Also, the Chernobyl releases occurred over about 10 days, while releases from Fukushima continued over a longer period of time. Mr. Tupin

Observational Evaluation of Simulated Land-Atmosphere Coupling on the U.S. Southern Great Plains

NASA Astrophysics Data System (ADS)

Phillips, T. J.; Klein, S. A.

2014-12-01

In a recent study of observed features of land-atmosphere coupling (LAC) at the ARM Southern Great Plains (ARM SGP) site in northern Oklahoma (Phillips and Klein, 2014 Journal of Geophysical Research), we identified statistically significant interactions between 1997-2008 summertime daily averages of soil moisture (at 10 cm depth) and a number of surface atmospheric variables, such as surface evaporation, relative humidity, and temperature. Here we will report on an evaluation of similar features of LAC simulated by version 5 of the global Community Atmosphere Model (CAM5), coupled to its native CLM4 land model, and downscaled to the vicinity of the ARM SGP site. In these case studies, the CAM5 was initialized from a 6-hourly atmospheric reanalysis for each day of the years 2008 and 2009 (where the CLM4 land state was equilibrated to the atmospheric model state), thus permitting a close comparison of the modeled and observed summer daily average features of the LAC in these years. Correlation coefficients R and "sensitivity indices" I (a measure of the comparative change of an atmospheric variable for a one-standard-deviation change in soil moisture) provided quantitative measures of the respective coupling strengths. Such a comparison of observed versus modeled LAC is complicated by differences in atmospheric forcings of the land; for example, the CAM5's summertime precipitation is too scant, and thus the model's upper soil layer often is drier than observed. The modeled daily average covariations of soil moisture with lower atmospheric variables also display less coherence (lower R values), but sometimes greater "sensitivity" (higher I values) than are observed at the ARM SGP site. Since the observational estimate of LAC may itself be sensitive to soil moisture measurement biases, we also will report on a planned investigation of the dependence of LAC on several alternative choices of soil moisture data sets local to the ARM SGP site. AcknowledgmentsThis work was funded by the U.S. Department of Energy Office of Science and was performed at the Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

Impact of air-sea drag coefficient for latent heat flux on large scale climate in coupled and atmosphere stand-alone simulations

NASA Astrophysics Data System (ADS)

Torres, Olivier; Braconnot, Pascale; Marti, Olivier; Gential, Luc

2018-05-01

The turbulent fluxes across the ocean/atmosphere interface represent one of the principal driving forces of the global atmospheric and oceanic circulation. Despite decades of effort and improvements, representation of these fluxes still presents a challenge due to the small-scale acting turbulent processes compared to the resolved scales of the models. Beyond this subgrid parameterization issue, a comprehensive understanding of the impact of air-sea interactions on the climate system is still lacking. In this paper we investigates the large-scale impacts of the transfer coefficient used to compute turbulent heat fluxes with the IPSL-CM4 climate model in which the surface bulk formula is modified. Analyzing both atmosphere and coupled ocean-atmosphere general circulation model (AGCM, OAGCM) simulations allows us to study the direct effect and the mechanisms of adjustment to this modification. We focus on the representation of latent heat flux in the tropics. We show that the heat transfer coefficients are highly similar for a given parameterization between AGCM and OAGCM simulations. Although the same areas are impacted in both kind of simulations, the differences in surface heat fluxes are substantial. A regional modification of heat transfer coefficient has more impact than uniform modification in AGCM simulations while in OAGCM simulations, the opposite is observed. By studying the global energetics and the atmospheric circulation response to the modification, we highlight the role of the ocean in dampening a large part of the disturbance. Modification of the heat exchange coefficient modifies the way the coupled system works due to the link between atmospheric circulation and SST, and the different feedbacks between ocean and atmosphere. The adjustment that takes place implies a balance of net incoming solar radiation that is the same in all simulations. As there is no change in model physics other than drag coefficient, we obtain similar latent heat flux between coupled simulations with different atmospheric circulations. Finally, we analyze the impact of model tuning and show that it can offset part of the feedbacks.

Exploring the Lyapunov instability properties of high-dimensional atmospheric and climate models

NASA Astrophysics Data System (ADS)

De Cruz, Lesley; Schubert, Sebastian; Demaeyer, Jonathan; Lucarini, Valerio; Vannitsem, Stéphane

2018-05-01

The stability properties of intermediate-order climate models are investigated by computing their Lyapunov exponents (LEs). The two models considered are PUMA (Portable University Model of the Atmosphere), a primitive-equation simple general circulation model, and MAOOAM (Modular Arbitrary-Order Ocean-Atmosphere Model), a quasi-geostrophic coupled ocean-atmosphere model on a β-plane. We wish to investigate the effect of the different levels of filtering on the instabilities and dynamics of the atmospheric flows. Moreover, we assess the impact of the oceanic coupling, the dissipation scheme, and the resolution on the spectra of LEs. The PUMA Lyapunov spectrum is computed for two different values of the meridional temperature gradient defining the Newtonian forcing to the temperature field. The increase in the gradient gives rise to a higher baroclinicity and stronger instabilities, corresponding to a larger dimension of the unstable manifold and a larger first LE. The Kaplan-Yorke dimension of the attractor increases as well. The convergence rate of the rate function for the large deviation law of the finite-time Lyapunov exponents (FTLEs) is fast for all exponents, which can be interpreted as resulting from the absence of a clear-cut atmospheric timescale separation in such a model. The MAOOAM spectra show that the dominant atmospheric instability is correctly represented even at low resolutions. However, the dynamics of the central manifold, which is mostly associated with the ocean dynamics, is not fully resolved because of its associated long timescales, even at intermediate orders. As expected, increasing the mechanical atmosphere-ocean coupling coefficient or introducing a turbulent diffusion parametrisation reduces the Kaplan-Yorke dimension and Kolmogorov-Sinai entropy. In all considered configurations, we are not yet in the regime in which one can robustly define large deviation laws describing the statistics of the FTLEs. This paper highlights the need to investigate the natural variability of the atmosphere-ocean coupled dynamics by associating rate of growth and decay of perturbations with the physical modes described using the formalism of the covariant Lyapunov vectors and considering long integrations in order to disentangle the dynamical processes occurring at all timescales.

Diagnosing the Nature of Land-Atmosphere Coupling During the 2006-7 Dry/Wet Extremes in the U. S. Southern Great Plains

NASA Technical Reports Server (NTRS)

Santanello, Joseph A., Jr.; Peters-Lidard, Christa D.; Kumar, Sujay V.; Dong, Xiquan; Kennedy, Aaron D.

2011-01-01

The degree of coupling between the land surface and PBL in NWP models remains largely undiagnosed due to the complex interactions and feedbacks present across a range of scales. In this study, a framework for diagnosing local land-atmosphere coupling (LoCo) is presented using a coupled mesoscale model with observations during the summers of 2006/7 in the U.S. Southern Great Plains. Specifically, the Weather Research and Forecasting (WRF) model has been coupled to NASA's Land Information System (LIS), which enables a suite of PBL and land surface model (LSM) options along provides a flexible and high-resolution representation and initialization of land surface physics and states. This coupling is one component of a larger project to develop a NASA-Unified WRF (NU-WRF) system. A range of diagnostics exploring the feedbacks between soil moisture and precipitation are examined for the dry/wet extremes, along with the sensitivity of PBL-LSM coupling to perturbations in soil moisture.

Observations and High-Resolution Numerical Simulations of a Non-Developing Tropical Disturbance in the Western North Pacific

DTIC Science & Technology

2013-09-01

potential energy CFSR Climate Forecast System Reanalysis COAMPS Coupled Ocean / Atmosphere Mesoscale Prediction System DA data assimilation DART Data...developing (TCS025) tropical disturbance using the adjoint and tangent linear models for the Coupled Ocean – Atmosphere Mesoscale Prediction System (COAMPS...for Medium-range Weather Forecasts ELDORA ELectra DOppler RAdar EOL Earth Observing Laboratory GPS global positioning system GTS Global

Utility of Satellite Remote Sensing for Land-Atmosphere Coupling and Drought Metrics

NASA Technical Reports Server (NTRS)

Roundy, Joshua K.; Santanello, Joseph A.

2017-01-01

Feedbacks between the land and the atmosphere can play an important role in the water cycle and a number of studies have quantified Land-Atmosphere (L-A) interactions and feedbacks through observations and prediction models. Due to the complex nature of L-A interactions, the observed variables are not always available at the needed temporal and spatial scales. This work derives the Coupling Drought Index (CDI) solely from satellite data and evaluates the input variables and the resultant CDI against in-situ data and reanalysis products. NASA's AQUA satellite and retrievals of soil moisture and lower tropospheric temperature and humidity properties are used as input. Overall, the AQUA-based CDI and its inputs perform well at a point, spatially, and in time (trends) compared to in-situ and reanalysis products. In addition, this work represents the first time that in-situ observations were utilized for the coupling classification and CDI. The combination of in-situ and satellite remote sensing CDI is unique and provides an observational tool for evaluating models at local and large scales. Overall, results indicate that there is sufficient information in the signal from simultaneous measurements of the land and atmosphere from satellite remote sensing to provide useful information for applications of drought monitoring and coupling metrics.

Utility of Satellite Remote Sensing for Land-Atmosphere Coupling and Drought Metrics

PubMed Central

Roundy, Joshua K.; Santanello, Joseph A.

2018-01-01

Feedbacks between the land and the atmosphere can play an important role in the water cycle and a number of studies have quantified Land-Atmosphere (L-A) interactions and feedbacks through observations and prediction models. Due to the complex nature of L-A interactions, the observed variables are not always available at the needed temporal and spatial scales. This work derives the Coupling Drought Index (CDI) solely from satellite data and evaluates the input variables and the resultant CDI against in-situ data and reanalysis products. NASA’s AQUA satellite and retrievals of soil moisture and lower tropospheric temperature and humidity properties are used as input. Overall, the AQUA-based CDI and its inputs perform well at a point, spatially, and in time (trends) compared to in-situ and reanalysis products. In addition, this work represents the first time that in-situ observations were utilized for the coupling classification and CDI. The combination of in-situ and satellite remote sensing CDI is unique and provides an observational tool for evaluating models at local and large scales. Overall, results indicate that there is sufficient information in the signal from simultaneous measurements of the land and atmosphere from satellite remote sensing to provide useful information for applications of drought monitoring and coupling metrics. PMID:29645012

Eastern equatorial Pacific sea surface temperature annual cycle in the Kiel climate model: simulation benefits from enhancing atmospheric resolution

NASA Astrophysics Data System (ADS)

Wengel, C.; Latif, M.; Park, W.; Harlaß, J.; Bayr, T.

2018-05-01

A long-standing difficulty of climate models is to capture the annual cycle (AC) of eastern equatorial Pacific (EEP) sea surface temperature (SST). In this study, we first examine the EEP SST AC in a set of integrations of the coupled Kiel Climate Model, in which only atmosphere model resolution differs. When employing coarse horizontal and vertical atmospheric resolution, significant biases in the EEP SST AC are observed. These are reflected in an erroneous timing of the cold tongue's onset and termination as well as in an underestimation of the boreal spring warming amplitude. A large portion of these biases are linked to a wrong simulation of zonal surface winds, which can be traced back to precipitation biases on both sides of the equator and an erroneous low-level atmospheric circulation over land. Part of the SST biases also is related to shortwave radiation biases related to cloud cover biases. Both wind and cloud cover biases are inherent to the atmospheric component, as shown by companion uncoupled atmosphere model integrations forced by observed SSTs. Enhancing atmosphere model resolution, horizontal and vertical, markedly reduces zonal wind and cloud cover biases in coupled as well as uncoupled mode and generally improves simulation of the EEP SST AC. Enhanced atmospheric resolution reduces convection biases and improves simulation of surface winds over land. Analysis of a subset of models from the Coupled Model Intercomparison Project phase 5 (CMIP5) reveals that in these models, very similar mechanisms are at work in driving EEP SST AC biases.

How robust is the atmospheric circulation response to Arctic sea-ice loss in isolation?

NASA Astrophysics Data System (ADS)

Kushner, P. J.; Hay, S. E.; Blackport, R.; McCusker, K. E.; Oudar, T.

2017-12-01

It is now apparent that active dynamical coupling between the ocean and atmosphere determines a good deal of how Arctic sea-ice loss changes the large-scale atmospheric circulation. In coupled ocean-atmosphere models, Arctic sea-ice loss indirectly induces a 'mini' global warming and circulation changes that extend into the tropics and the Southern Hemisphere. Ocean-atmosphere coupling also amplifies by about 50% Arctic free-tropospheric warming arising from sea-ice loss (Deser et al. 2015, 2016). The mechanisms at work and how to separate the response to sea-ice loss from the rest of the global warming process remain poorly understood. Different studies have used distinctive numerical approaches and coupled ocean-atmosphere models to address this problem. We put these studies on comparable footing using pattern scaling (Blackport and Kushner 2017) to separately estimate the part of the circulation response that scales with sea-ice loss in the absence of low-latitude warming from the part that scales with low-latitude warming in the absence of sea-ice loss. We consider well-sampled simulations from three different coupled ocean-atmosphere models (CESM1, CanESM2, CNRM-CM5), in which greenhouse warming and sea-ice loss are driven in different ways (sea ice albedo reduction/transient RCP8.5 forcing for CESM1, nudged sea ice/CO2 doubling for CanESM2, heat-flux forcing/constant RCP8.5-derived forcing for CNRM-CM5). Across these different simulations, surprisingly robust influences of Arctic sea-ice loss on atmospheric circulation can be diagnosed using pattern scaling. For boreal winter, the isolated sea-ice loss effect acts to increase warming in the North American Sub-Arctic, decrease warming of the Eurasian continent, enhance precipitation over the west coast of North America, and strengthen the Aleutian Low and the Siberian High. We will also discuss how Arctic free tropospheric warming might be enhanced via midlatitude ocean surface warming induced by sea-ice loss. Less robust is the part of the response that scales with low-latitude warming, which, depending on the model, can reinforce or cancel the response to sea-ice loss. The extent to which a "tug of war" exists between tropical and high-latitude influences on the general circulation might thus be model dependent.

Underground Nuclear Explosions and Release of Radioactive Noble Gases

NASA Astrophysics Data System (ADS)

Dubasov, Yuri V.

2010-05-01

Over a period in 1961-1990 496 underground nuclear tests and explosions of different purpose and in different rocks were conducted in the Soviet Union at Semipalatinsk and anovaya Zemlya Test Sites. A total of 340 underground nuclear tests were conducted at the Semipalatinsk Test Site. One hundred seventy-nine explosions (52.6%) among them were classified as these of complete containment, 145 explosions (42.6%) as explosions with weak release of radioactive noble gases (RNG), 12 explosions (3.5%) as explosions with nonstandard radiation situation, and four excavation explosions with ground ejection (1.1%). Thirty-nine nuclear tests had been conducted at the Novaya Zemlya Test Site; six of them - in shafts. In 14 tests (36%) there were no RNG release. Twenty-three tests have been accompanied by RNG release into the atmosphere without sedimental contamination. Nonstandard radiation situation occurred in two tests. In incomplete containment explosions both early-time RNG release (up to ~1 h) and late-time release from 1 to 28 h after the explosion were observed. Sometimes gas release took place for several days, and it occurred either through tunnel portal or epicentral zone, depending on atmospheric air temperature.

Ca2+ Entry is Required for Mechanical Stimulation-induced ATP Release from Astrocyte

PubMed Central

Lee, Jaekwang; Chun, Ye-Eun; Han, Kyung-Seok; Lee, Jungmoo; Woo, Dong Ho

2015-01-01

Astrocytes and neurons are inseparable partners in the brain. Neurotransmitters released from neurons activate corresponding G protein-coupled receptors (GPCR) expressed in astrocytes, resulting in release of gliotransmitters such as glutamate, D-serine, and ATP. These gliotransmitters in turn influence neuronal excitability and synaptic activities. Among these gliotransmitters, ATP regulates the level of network excitability and is critically involved in sleep homeostasis and astrocytic Ca2+ oscillations. ATP is known to be released from astrocytes by Ca2+-dependent manner. However, the precise source of Ca2+, whether it is Ca2+ entry from outside of cell or from the intracellular store, is still not clear yet. Here, we performed sniffer patch to detect ATP release from astrocyte by using various stimulation. We found that ATP was not released from astrocyte when Ca2+ was released from intracellular stores by activation of Gαq-coupled GPCR including PAR1, P2YR, and B2R. More importantly, mechanical stimulation (MS)-induced ATP release from astrocyte was eliminated when external Ca2+ was omitted. Our results suggest that Ca2+ entry, but not release from intracellular Ca2+ store, is critical for MS-induced ATP release from astrocyte. PMID:25792866

The total release of xenon-133 from the Fukushima Dai-ichi nuclear power plant accident.

PubMed

Stohl, Andreas; Seibert, Petra; Wotawa, Gerhard

2012-10-01

The accident at the Fukushima Dai-ichi nuclear power plant (FD-NPP) on 11 March 2011 released large amounts of radioactivity into the atmosphere. We determine the total emission of the noble gas xenon-133 ((133)Xe) using global atmospheric concentration measurements. For estimating the emissions, we used three different methods: (i) using a purely observation-based multi-box model, (ii) comparisons of dispersion model results driven with GFS meteorological data with the observation data, and (iii) such comparisons with the dispersion model driven by ECMWF data. From these three methods, we have obtained total (133)Xe releases from FD-NPP of (i) 16.7 ± 1.9 EBq, (ii) 14.2 ± 0.8 EBq, and (iii) 19.0 ± 3.4 EBq, respectively. These values are substantially larger than the entire (133)Xe inventory of FD-NPP of about 12.2 EBq derived from calculations of nuclear fuel burn-up. Complete release of the entire (133)Xe inventory of FD-NPP and additional release of (133)Xe due to the decay of iodine-133 ((133)I), which can add another 2 EBq to the (133)Xe FD-NPP inventory, is required to explain the atmospheric observations. Two of our three methods indicate even higher emissions, but this may not be a robust finding given the differences between our estimates. Copyright © 2012 Elsevier Ltd. All rights reserved.

Coupled Inertial Navigation and Flush Air Data Sensing Algorithm for Atmosphere Estimation

NASA Technical Reports Server (NTRS)

Karlgaard, Christopher D.; Kutty, Prasad; Schoenenberger, Mark

2015-01-01

This paper describes an algorithm for atmospheric state estimation that is based on a coupling between inertial navigation and flush air data sensing pressure measurements. In this approach, the full navigation state is used in the atmospheric estimation algorithm along with the pressure measurements and a model of the surface pressure distribution to directly estimate atmospheric winds and density using a nonlinear weighted least-squares algorithm. The approach uses a high fidelity model of atmosphere stored in table-look-up form, along with simplified models of that are propagated along the trajectory within the algorithm to provide prior estimates and covariances to aid the air data state solution. Thus, the method is essentially a reduced-order Kalman filter in which the inertial states are taken from the navigation solution and atmospheric states are estimated in the filter. The algorithm is applied to data from the Mars Science Laboratory entry, descent, and landing from August 2012. Reasonable estimates of the atmosphere and winds are produced by the algorithm. The observability of winds along the trajectory are examined using an index based on the discrete-time observability Gramian and the pressure measurement sensitivity matrix. The results indicate that bank reversals are responsible for adding information content to the system. The algorithm is then applied to the design of the pressure measurement system for the Mars 2020 mission. The pressure port layout is optimized to maximize the observability of atmospheric states along the trajectory. Linear covariance analysis is performed to assess estimator performance for a given pressure measurement uncertainty. The results indicate that the new tightly-coupled estimator can produce enhanced estimates of atmospheric states when compared with existing algorithms.

NESHAP Area-Specific Dose-Release Factors for Potential Onsite Member-of-the-Public Locations at SRS using CAP88-PC Version 4.0

DOE Office of Scientific and Technical Information (OSTI.GOV)

Trimor, P.

The Environmental Protection Agency (EPA) requires the use of the computer model CAP88-PC to estimate the total effective doses (TED) for demonstrating compliance with 40 CFR 61, Subpart H (EPA 2006), the National Emission Standards for Hazardous Air Pollutants (NESHAP) regulations. As such, CAP88 Version 4.0 was used to calculate the receptor dose due to routine atmospheric releases at the Savannah River Site (SRS). For estimation, NESHAP dose-release factors (DRFs) have been supplied to Environmental Compliance and Area Closure Projects (EC&ACP) for many years. DRFs represent the dose to a maximum receptor exposed to 1 Ci of a specified radionuclidemore » being released into the atmosphere. They are periodically updated to include changes in the CAP88 version, input parameter values, site meteorology, and location of the maximally exposed individual (MEI). In this report, the DRFs were calculated for potential radionuclide atmospheric releases from 13 SRS release points. The three potential onsite MEI locations to be evaluated are B-Area, Three Rivers Landfill (TRL), and Savannah River Ecology Lab Conference Center (SRELCC) with TRL’s onsite workers considered as members-of-the-public, and the potential future constructions of dormitories at SRELCC and Barracks at B-Area. Each MEI location was evaluated at a specified compass sector with different area to receptor distances and was conducted for both ground-level and elevated release points. The analysis makes use of area-specific meteorological data (Viner 2014). The resulting DRFs are compared to the 2014 NESHAP offsite MEI DRFs for three operational areas; A-Area, H-Area, and COS for a release rate of 1 Ci of tritium oxide at 0 ft. elevation. CAP88 was executed again using the 2016 NESHAP MEI release rates for 0 and 61 m stack heights to determine the radionuclide dose at TRL from the center-of-site (COS).« less

Effects of elevated atmospheric Co2 and tropospheric O3 on nutrient dynamics: decomposition of leaf litter in trembling aspen and paper birch communities. Plant Soil. 299:65–82.

Treesearch

Lingli Liu; John S. King; Christian P. Giardina

2007-01-01

Atmospheric changes could strongly influence how terrestrial ecosystems function by altering nutrient cycling. We examined how the dynamics of nutrient release from leaf litter responded to two important atmospheric changes: rising atmospheric Co2 and tropospheric O3. We evaluated the independent and combined effects of...

Volatile Transport by Volcanic Plumes on Earth, Venus and Mars

NASA Technical Reports Server (NTRS)

Glaze, Lori S.; Self, Stephen; Baloga, Steve; Stofan, Ellen R.

2012-01-01

Explosive volcanic eruptions can produce sustained, buoyant columns of ash and gas in the atmosphere (Fig. 1). Large flood basalt eruptions may also include significant explosive phases that generate eruption columns. Such eruptions can transport volcanic volatiles to great heights in the atmosphere. Volcanic eruption columns can also redistribute chemical species within the atmosphere by entraining ambient atmosphere at low altitudes and releasing those species at much higher altitudes.

First retrieval of hourly atmospheric radionuclides just after the Fukushima accident by analyzing filter-tapes of operational air pollution monitoring stations.

PubMed

Tsuruta, Haruo; Oura, Yasuji; Ebihara, Mitsuru; Ohara, Toshimasa; Nakajima, Teruyuki

2014-10-22

No observed data have been found in the Fukushima Prefecture (FP) for the time-series of atmospheric radionuclides concentrations just after the Fukushima Daiichi Nuclear Power Plant (FD1NPP) accident. Accordingly, current estimates of internal radiation doses from inhalation, and atmospheric radionuclide concentrations by atmospheric transport models are highly uncertain. Here, we present a new method for retrieving the hourly atmospheric (137)Cs concentrations by measuring the radioactivity of suspended particulate matter (SPM) collected on filter tapes in SPM monitors which were operated even after the accident. This new dataset focused on the period of March 12-23, 2011 just after the accident, when massive radioactive materials were released from the FD1NPP to the atmosphere. Overall, 40 sites of the more than 400 sites in the air quality monitoring stations in eastern Japan were studied. For the first time, we show the spatio-temporal variation of atmospheric (137)Cs concentrations in the FP and the Tokyo Metropolitan Area (TMA) located more than 170 km southwest of the FD1NPP. The comprehensive dataset revealed how the polluted air masses were transported to the FP and TMA, and can be used to re-evaluate internal exposure, time-series radionuclides release rates, and atmospheric transport models.

Where do winds come from? A new theory on how water vapor condensation influences atmospheric pressure and dynamics

NASA Astrophysics Data System (ADS)

Makarieva, A. M.; Gorshkov, V. G.; Sheil, D.; Nobre, A. D.; Li, B.-L.

2013-01-01

Phase transitions of atmospheric water play a ubiquitous role in the Earth's climate system, but their direct impact on atmospheric dynamics has escaped wide attention. Here we examine and advance a theory as to how condensation influences atmospheric pressure through the mass removal of water from the gas phase with a simultaneous account of the latent heat release. Building from fundamental physical principles we show that condensation is associated with a decline in air pressure in the lower atmosphere. This decline occurs up to a certain height, which ranges from 3 to 4 km for surface temperatures from 10 to 30 °C. We then estimate the horizontal pressure differences associated with water vapor condensation and find that these are comparable in magnitude with the pressure differences driving observed circulation patterns. The water vapor delivered to the atmosphere via evaporation represents a store of potential energy available to accelerate air and thus drive winds. Our estimates suggest that the global mean power at which this potential energy is released by condensation is around one per cent of the global solar power - this is similar to the known stationary dissipative power of general atmospheric circulation. We conclude that condensation and evaporation merit attention as major, if previously overlooked, factors in driving atmospheric dynamics.

Insights in time dependent cross compartment sensitivities from ensemble simulations with the fully coupled subsurface-land surface-atmosphere model TerrSysMP

NASA Astrophysics Data System (ADS)

Schalge, Bernd; Rihani, Jehan; Haese, Barbara; Baroni, Gabriele; Erdal, Daniel; Haefliger, Vincent; Lange, Natascha; Neuweiler, Insa; Hendricks-Franssen, Harrie-Jan; Geppert, Gernot; Ament, Felix; Kollet, Stefan; Cirpka, Olaf; Saavedra, Pablo; Han, Xujun; Attinger, Sabine; Kunstmann, Harald; Vereecken, Harry; Simmer, Clemens

2017-04-01

Currently, an integrated approach to simulating the earth system is evolving where several compartment models are coupled to achieve the best possible physically consistent representation. We used the model TerrSysMP, which fully couples subsurface, land surface and atmosphere, in a synthetic study that mimicked the Neckar catchment in Southern Germany. A virtual reality run at a high resolution of 400m for the land surface and subsurface and 1.1km for the atmosphere was made. Ensemble runs at a lower resolution (800m for the land surface and subsurface) were also made. The ensemble was generated by varying soil and vegetation parameters and lateral atmospheric forcing among the different ensemble members in a systematic way. It was found that the ensemble runs deviated for some variables and some time periods largely from the virtual reality reference run (the reference run was not covered by the ensemble), which could be related to the different model resolutions. This was for example the case for river discharge in the summer. We also analyzed the spread of model states as function of time and found clear relations between the spread and the time of the year and weather conditions. For example, the ensemble spread of latent heat flux related to uncertain soil parameters was larger under dry soil conditions than under wet soil conditions. Another example is that the ensemble spread of atmospheric states was more influenced by uncertain soil and vegetation parameters under conditions of low air pressure gradients (in summer) than under conditions with larger air pressure gradients in winter. The analysis of the ensemble of fully coupled model simulations provided valuable insights in the dynamics of land-atmosphere feedbacks which we will further highlight in the presentation.

Shape memory-based actuators and release mechanisms therefrom

NASA Technical Reports Server (NTRS)

Vaidyanathan, Rajan (Inventor); Snyder, Daniel W. (Inventor); Schoenwald, David K. (Inventor); Lam, Nhin S. (Inventor); Watson, Daniel S. (Inventor); Krishnan, Vinu B. (Inventor); Noebe, Ronald D. (Inventor)

2012-01-01

SM-based actuators (110) and release mechanisms (100) therefrom and systems (500) including one or more release mechanisms (100). The actuators (110) comprise a SM member (118) and a deformable member (140) mechanically coupled to the SM member (118) which deforms upon a shape change of the SM member triggered by a phase transition of the SM member. A retaining element (160) is mechanically coupled to the deformable member (140), wherein the retaining element (160) moves upon the shape change. Release mechanism (100) include an actuator, a rotatable mechanism (120) including at least one restraining feature (178) for restraining rotational movement of the retaining element (160) before the shape change, and at least one spring (315) that provides at least one locked spring-loaded position when the retaining element is in the restraining feature and at least one released position that is reached when the retaining element is in a position beyond the restraining feature (178). The rotatable mechanism (120) includes at least one load-bearing protrusion (310). A hitch (400) is for mechanically coupling to the load, wherein the hitch is supported on the load bearing protrusion (310) when the rotatable mechanism is in the locked spring-loaded position.

Impact-Mobilized Dust in the Martian Atmosphere

NASA Technical Reports Server (NTRS)

Nemtchinov, I. V.; Shuvalov, V. V.; Greeley, R.

2002-01-01

We consider dust production and entrainment into the atmosphere of Mars by impacts. Numerical simulations based on the multidimensional multimaterial hydrocode were conducted for impactors 1 to 100 m in size and velocities 11 and 20 kilometers per second. The size distribution of particles was based on experimentrr wing TNT explosions. Dust can be mobilized even when the impactor does not reach the ground through the release of energy in the atmosphere, We found that the blast produced winds entrained dust by a mechanism similar to boundary layer winds as determined from the wind-tunnel tests. For a l-m radius stony asteroid releasing its energy in the atmosphere the lifted mass of dust is larger than that in a typical dust devil and could trigger local dust storms, For a 100-m-radius meteoroid the amount of injected dust is comparable with the tota! mass of a global dust storm.

The role of precipitation in aerosol-induced changes in northern hemisphere wintertime stationary waves

NASA Astrophysics Data System (ADS)

Lewinschal, A.; Ekman, A. M. L.; Körnich, H.

2012-04-01

Aerosol particles have a considerable impact on the energy budget of the atmosphere due to their ability to scatter and absorb incoming solar radiation. Persistent particle emissions in certain regions of the world have lead to quasi-permanent aerosol forcing patterns. This spatially varying forcing pattern has the potential to modify temperature gradients that in turn alter pressure gradients and the atmospheric circulation. This study focuses on the effect of aerosol direct radiative forcing on northern hemisphere wintertime stationary waves. A global general circulation model based on the ECMWF operational forecast model is applied (EC-Earth). Aerosols are prescribed as monthly mean mixing ratios of sulphate, black carbon, organic carbon, dust and sea salt. Only the direct aerosol effect is considered. The climatic change is defined as the difference between model simulations using present-day and pre-industrial concentrations of aerosol particles. Data from 40-year long simulations using a coupled ocean-atmosphere model system are used. In EC-Earth, the high aerosol loading over South Asia leads to a surface cooling, which appears to enhance the South Asian winter monsoon and weaken the Indian Ocean Walker circulation. The anomalous Walker circulation leads to changes in tropical convective precipitation and consequent changes in latent heat release which effectively acts to generate planetary scale waves propagating into the extra-tropics. Using a steady-state linear model we verify that the aerosol-induced anomalous convective precipitation is a crucial link between the wave changes and the direct aerosol radiative forcing.

Upper atmosphere has cooled steadily for three decades

NASA Astrophysics Data System (ADS)

Wendel, JoAnna

2014-11-01

Increasing amounts of greenhouse gases released by human activities do not just affect only the lower atmosphere: Scientists project that anthropogenic carbon emissions have caused a cooling trend in the upper atmosphere, between 200 and 400 kilometers, over the past few decades. Cooling in this atmospheric region can affect the operations of satellites and the orbits of space junk. However, data about cooling trends in the upper atmosphere are still incomplete, and better data are needed to confirm this projection.

Lift and Power Required for Flapping Wing Hovering Flight on Mars

NASA Astrophysics Data System (ADS)

Pohly, Jeremy; Sridhar, Madhu; Bluman, James; Kang, Chang-Kwon; Landrum, D. Brian; Fahimi, Farbod; Aono, Hikaru; Liu, Hao

2017-11-01

Achieving flight on Mars is challenging due to the ultra-low density atmosphere. Bio-inspired flapping motion can generate sufficient lift if bumblebee-inspired wings are scaled up between 2 and 4 times their nominal size. However, due to this scaling, the inertial power required to sustain hover increases and dominates over the aerodynamic power. Our results show that a torsional spring placed at the wing root can reduce the flapping power required for hover by efficiently storing and releasing energy while operating at its resonance frequency. The spring assisted reduction in flapping power is demonstrated with a well-validated, coupled Navier-Stokes and flight dynamics solver. The total power is reduced by 79%, whereas the flapping power is reduced by 98%. Such a reduction in power paves the way for an efficient, realizable micro air vehicle capable of vertical takeoff and landing as well as sustained flight on Mars. Alabama Space Grant Consortium Fellowship.

The marine geological record of industrialization

NASA Astrophysics Data System (ADS)

Ridgwell, A.

2007-12-01

In the far distant future, what traces of our industrialized civilization could a hypothetical alien visitor to the Earth identify our ever having existed by? Popular perception is of landfills being excavated and species extinctions identified. However, localized terrestrial deposits and loss of only a relatively small proportion of species would be fickle candidates for reliable preservation in the geological record. Rather, the imprint of our current civilization will be seen in a global-scale dissolution-preservation event of carbonate in marine sediments, coupled to a pronounced negative carbon isotopic excursion. This is the geological fingerprint of massive carbon release to the oceans and atmosphere in injunction with the rock weathering consequences of a global warming transient. In this contribution I explore the characteristics of the future marine geological record of industrialization and draw parallels with observations recorded in sediments spanning the Paleocene-Eocene Thermal Maximum.

TOWARDS OPERATIONAL FORECASTING OF LOWER ATMOSPHERE EFFECTS ON THE UPPER ATMOSPHERE AND IONOSPHERE: INTEGRATED DYNAMICS IN EARTH’S ATMOSPHERE (IDEA)

NASA Astrophysics Data System (ADS)

Akmaev, R. A.; Fuller-Rowell, T. J.; Wu, F.; Wang, H.; Juang, H.; Moorthi, S.; Iredell, M.

2009-12-01

The upper atmosphere and ionosphere exhibit variability and phenomena that have been associated with planetary and tidal waves originating in the lower atmosphere. To study and be able to predict the effects of these global-scale dynamical perturbations on the coupled thermosphere-ionosphere-electrodynamics system a new coupled model is being developed under the IDEA project. To efficiently cross the infamous R2O “death valley”, from the outset the IDEA project leverages the natural synergy between NOAA’s National Weather Service’s (NWS) Space Weather Prediction and Environmental Modeling Centers and a NOAA-University of Colorado cooperative institute (CIRES). IDEA interactively couples a Whole Atmosphere Model (WAM) with ionosphere-plasmasphere and electrodynamics models. WAM is a 150-layer general circulation model (GCM) based on NWS’s operational weather prediction Global Forecast System (GFS) extended from its nominal top altitude of 62 km to over 600 km. It incorporates relevant physical processes including those responsible for the generation of tidal and planetary waves in the troposphere and stratosphere. Long-term simulations reveal realistic seasonal variability of tidal waves with a substantial contribution from non-migrating tidal modes, recently implicated in the observed morphology of the ionosphere. Such phenomena as the thermospheric Midnight Temperature Maximum (MTM), previously associated with the tides, are also realistically simulated for the first time.

Photocatalytic thin films coupled with polymeric microcapsules for the controlled-release of volatile agents upon solar activation

NASA Astrophysics Data System (ADS)

Oliveira, L. F.; Marques, J.; Coutinho, P. J. G.; Parpot, P.; Tavares, C. J.

2013-06-01

This work reportson the application of solar-activated photocatalytic thin films that allow the controlled-release of volatile agents (e.g., insecticides, repellents) from the interior of adsorbedpolymericmicrocapsules. In order to standardize the tests, a quantification of the inherent controlled-release of a particular volatile agent is determined by gas chromatography coupled to mass spectroscopy, so that an application can be offered to a wide range of supports from various industrial sectors, such as in textiles (clothing, curtains, mosquito nets). This technology takes advantage of the established photocatalytic property of titanium dioxide (TiO2) for the use as an active surface/site to promote the controlled-release of a specific vapor (volatile agentfrom within the aforementioned microcapsules.

Tracing Acoustic-Gravity Waves from the Ocean into the Ionosphere

NASA Astrophysics Data System (ADS)

Zabotin, N. A.; Godin, O. A.; Bullett, T. W.; Negrea, C.

2013-12-01

Ionospheric manifestations of tsunamis provide dramatic evidence of a connection between wave processes in the ocean and in the atmosphere. But tsunamis are only a transient feature of a more general phenomenon, infragravity waves (IGWs). IGWs are permanently present surface gravity waves in the ocean with periods longer than the longest periods (~30 s) of wind-generated waves. IGWs propagate transoceanic distances and, because of their long wavelengths (from ~1 km to hundreds of km), provide a mechanism for coupling wave processes in the ocean, atmosphere, and the solid Earth. The notion that tsunamis may generate waves in the upper atmosphere has existed for a long time but no quantitative coupling theory for the background waves has been proposed. We provide a strict physical justification for the influence of the background IGWs on the upper atmosphere. Taking into account both fluid compressibility and the gravity in a coupled atmosphere-ocean system, we show that there exist two distinct regimes of IGW penetration into the atmosphere. At higher frequencies, one has evanescent waves in the atmosphere propagating horizontally along the ocean surface. At lower frequencies, IGWs continuously radiate their energy into the upper atmosphere in the form of acoustic gravity waves (AGWs). The transition frequency depends on the ocean depth; it varies slowly near 3 mHz for typical depth values and drops to zero sharply only for extremely large depths. Using semi-empirical model of the IGW power spectrum, we derive an estimate of the flux of the mechanical energy and mechanical momentum from the deep ocean into the atmosphere due to background IGWs and predict specific forcing on the atmosphere in coastal regions. We compare spectra of wave processes in the ionosphere measured using Dynasonde technique over Wallops Island, VA and San Juan, PR and interpret the differences in terms of the oceanic effects. We conclude that AGWs of oceanic origin may have an observable impact on the upper atmosphere and describe techniques for experimental verification of this finding.

Effects of atmospheric CO2 enrichment on soil CO2 efflux in a young longleaf pine system

Treesearch

G. Brett Runion; John R. Butnor; S. A. Prior; R. J. Mitchell; H. H. Rogers

2012-01-01

The southeastern landscape is composed of agricultural and forest systems that can store carbon (C) in standing biomass and soil. Research is needed to quantify the effects of elevated atmospheric carbon dioxide (CO2) on terrestrial C dynamics including CO2 release back to the atmosphere and soil sequestration. Longleaf...

Effects of Precipitation on Ocean Mixed-Layer Temperature and Salinity as Simulated in a 2-D Coupled Ocean-Cloud Resolving Atmosphere Model

NASA Technical Reports Server (NTRS)

Li, Xiaofan; Sui, C.-H.; Lau, K-M.; Adamec, D.

1999-01-01

A two-dimensional coupled ocean-cloud resolving atmosphere model is used to investigate possible roles of convective scale ocean disturbances induced by atmospheric precipitation on ocean mixed-layer heat and salt budgets. The model couples a cloud resolving model with an embedded mixed layer-ocean circulation model. Five experiment are performed under imposed large-scale atmospheric forcing in terms of vertical velocity derived from the TOGA COARE observations during a selected seven-day period. The dominant variability of mixed-layer temperature and salinity are simulated by the coupled model with imposed large-scale forcing. The mixed-layer temperatures in the coupled experiments with 1-D and 2-D ocean models show similar variations when salinity effects are not included. When salinity effects are included, however, differences in the domain-mean mixed-layer salinity and temperature between coupled experiments with 1-D and 2-D ocean models could be as large as 0.3 PSU and 0.4 C respectively. Without fresh water effects, the nocturnal heat loss over ocean surface causes deep mixed layers and weak cooling rates so that the nocturnal mixed-layer temperatures tend to be horizontally-uniform. The fresh water flux, however, causes shallow mixed layers over convective areas while the nocturnal heat loss causes deep mixed layer over convection-free areas so that the mixed-layer temperatures have large horizontal fluctuations. Furthermore, fresh water flux exhibits larger spatial fluctuations than surface heat flux because heavy rainfall occurs over convective areas embedded in broad non-convective or clear areas, whereas diurnal signals over whole model areas yield high spatial correlation of surface heat flux. As a result, mixed-layer salinities contribute more to the density differences than do mixed-layer temperatures.

The GEOS-5 Atmospheric General Circulation Model: Mean Climate and Development from MERRA to Fortuna

NASA Technical Reports Server (NTRS)

Molod, Andrea; Takacs, Lawrence; Suarez, Max; Bacmeister, Julio; Song, In-Sun; Eichmann, Andrew

2012-01-01

This report is a documentation of the Fortuna version of the GEOS-5 Atmospheric General Circulation Model (AGCM). The GEOS-5 AGCM is currently in use in the NASA Goddard Modeling and Assimilation Office (GMAO) for simulations at a wide range of resolutions, in atmosphere only, coupled ocean-atmosphere, and data assimilation modes. The focus here is on the development subsequent to the version that was used as part of NASA s Modern-Era Retrospective Analysis for Research and Applications (MERRA). We present here the results of a series of 30-year atmosphere-only simulations at different resolutions, with focus on the behavior of the 1-degree resolution simulation. The details of the changes in parameterizations subsequent to the MERRA model version are outlined, and results of a series of 30-year, atmosphere-only climate simulations at 2-degree resolution are shown to demonstrate changes in simulated climate associated with specific changes in parameterizations. The GEOS-5 AGCM presented here is the model used for the GMAO s atmosphere-only and coupled CMIP-5 simulations.

Planetary Wave-Tide Interactions in Atmosphere-Ionosphere Coupling, Xiaoli Zhang, Jeffrey M. Forbes, Astrid Maute, and Maura E. Hagan

NASA Astrophysics Data System (ADS)

Zhang, X.; Forbes, J. M.; Maute, A. I.

2017-12-01

Planetary Wave-Tide Interactions in Atmosphere-Ionosphere Coupling Xiaoli Zhang, Jeffrey M. Forbes, Astrid Maute, and Maura E. Hagan The existence of secondary waves in the mesosphere and thermosphere due to nonlinear interactions between atmospheric tides and longer-period waves have been revealed in both satellite data and in the National Center for Atmospheric Research (NCAR) Thermosphere Ionosphere Mesosphere Electrodynamics General Circulation Model (TIME-GCM). The longer-period waves include the quasi-2-day and 6-day westward-propagating "normal modes" of the atmosphere, and eastward-propagating ultra-fast Kelvin waves with periods between 2 and 4 days. The secondary waves add to both the temporal and longitude variability of the atmosphere beyond that associated with the linear superposition of the interacting waves, thus adding "complexity" to the system. Based on our knowledge of the processes governing atmosphere-ionosphere interactions, similar revelations are expected to occur in electric fields, vertical plasma drifts and F-region electron densities. Towards this end, examples of such ionospheric manifestations of wave-wave interactions in TIE-GCM simulations will be presented.

Middle atmosphere electrical structure, dynamics and coupling

NASA Technical Reports Server (NTRS)

Hale, L. C.

1984-01-01

The ram current to ion traps and the insensitivity of ion conductivity to compressibility provide the basis of robust techniques for middle atmosphere measurements. Gerdien condensers are more difficult to implement but provide more information. Mesospheric electrical conductivity shows many orders of magnitude variability, with depressions below gas phase model values indicating dominance by aerosol particles. The mobility of these ions has been directly measured and indicates particles of thousands of AMU. Large mesospheric fields have come into question, and diagnostic measurements show that many such measurements may be artifacts. However, some measurements of V/m fields with symmetrical and redundant sensors appear to be real. These fields complicate the 'mapping' picture of electrical coupling and may also modulate the transport of aerosol particles. They are probably related to neutral atmospheric dynamics and/or the aerosol particles. Lightning couples much more energy to the middle atmosphere and above than previously suspected, primarily in the ELF-UHF range. There are many important unanswered questions in this relatively unexplored frontier area which may be answered with low cost balloon and sounding rocket experiments.

Congenital myopathy results from misregulation of a muscle Ca2+ channel by mutant Stac3

PubMed Central

Linsley, Jeremy W.; Hsu, I-Uen; Groom, Linda; Yarotskyy, Viktor; Lavorato, Manuela; Horstick, Eric J.; Linsley, Drew; Wang, Wenjia; Franzini-Armstrong, Clara; Dirksen, Robert T.; Kuwada, John Y.

2017-01-01

Skeletal muscle contractions are initiated by an increase in Ca2+ released during excitation–contraction (EC) coupling, and defects in EC coupling are associated with human myopathies. EC coupling requires communication between voltage-sensing dihydropyridine receptors (DHPRs) in transverse tubule membrane and Ca2+ release channel ryanodine receptor 1 (RyR1) in the sarcoplasmic reticulum (SR). Stac3 protein (SH3 and cysteine-rich domain 3) is an essential component of the EC coupling apparatus and a mutation in human STAC3 causes the debilitating Native American myopathy (NAM), but the nature of how Stac3 acts on the DHPR and/or RyR1 is unknown. Using electron microscopy, electrophysiology, and dynamic imaging of zebrafish muscle fibers, we find significantly reduced DHPR levels, functionality, and stability in stac3 mutants. Furthermore, stac3NAM myofibers exhibited increased caffeine-induced Ca2+ release across a wide range of concentrations in the absence of altered caffeine sensitivity as well as increased Ca2+ in internal stores, which is consistent with increased SR luminal Ca2+. These findings define critical roles for Stac3 in EC coupling and human disease. PMID:28003463

Sensitivity of global and regional terrestrial carbon storage to the direct CO2 effect and climate change based on the CMIP5 model intercomparison.

PubMed

Peng, Jing; Dan, Li; Huang, Mei

2014-01-01

Global and regional land carbon storage has been significantly affected by increasing atmospheric CO2 concentration and climate change. Based on fully coupled climate-carbon-cycle simulations from the Coupled Model Intercomparison Project Phase 5 (CMIP5), we investigate sensitivities of land carbon storage to rising atmospheric CO2 concentration and climate change over the world and 21 regions during the 130 years. Overall, the simulations suggest that consistently spatial positive effects of the increasing CO2 concentrations on land carbon storage are expressed with a multi-model averaged value of 1.04 PgC per ppm. The stronger positive values are mainly located in the broad areas of temperate and tropical forest, especially in Amazon basin and western Africa. However, large heterogeneity distributed for sensitivities of land carbon storage to climate change. Climate change causes decrease in land carbon storage in most tropics and the Southern Hemisphere. In these regions, decrease in soil moisture (MRSO) and enhanced drought somewhat contribute to such a decrease accompanied with rising temperature. Conversely, an increase in land carbon storage has been observed in high latitude and altitude regions (e.g., northern Asia and Tibet). The model simulations also suggest that global negative impacts of climate change on land carbon storage are predominantly attributed to decrease in land carbon storage in tropics. Although current warming can lead to an increase in land storage of high latitudes of Northern Hemisphere due to elevated vegetation growth, a risk of exacerbated future climate change may be induced due to release of carbon from tropics.

Sensitivity of Global and Regional Terrestrial Carbon Storage to the Direct CO2 Effect and Climate Change Based on the CMIP5 Model Intercomparison

PubMed Central

Peng, Jing; Dan, Li; Huang, Mei

2014-01-01

Global and regional land carbon storage has been significantly affected by increasing atmospheric CO2 concentration and climate change. Based on fully coupled climate-carbon-cycle simulations from the Coupled Model Intercomparison Project Phase 5 (CMIP5), we investigate sensitivities of land carbon storage to rising atmospheric CO2 concentration and climate change over the world and 21 regions during the 130 years. Overall, the simulations suggest that consistently spatial positive effects of the increasing CO2 concentrations on land carbon storage are expressed with a multi-model averaged value of 1.04PgC per ppm. The stronger positive values are mainly located in the broad areas of temperate and tropical forest, especially in Amazon basin and western Africa. However, large heterogeneity distributed for sensitivities of land carbon storage to climate change. Climate change causes decrease in land carbon storage in most tropics and the Southern Hemisphere. In these regions, decrease in soil moisture (MRSO) and enhanced drought somewhat contribute to such a decrease accompanied with rising temperature. Conversely, an increase in land carbon storage has been observed in high latitude and altitude regions (e.g., northern Asia and Tibet). The model simulations also suggest that global negative impacts of climate change on land carbon storage are predominantly attributed to decrease in land carbon storage in tropics. Although current warming can lead to an increase in land storage of high latitudes of Northern Hemisphere due to elevated vegetation growth, a risk of exacerbated future climate change may be induced due to release of carbon from tropics. PMID:24748331

Nonmigrating tidal impact on the CO2 15 μm infrared cooling of the lower thermosphere during solar minimum conditions

NASA Astrophysics Data System (ADS)

Nischal, N.; Oberheide, J.; Mlynczak, M. G.; Hunt, L. A.; Maute, A.

2017-06-01

Carbon dioxide (CO2) infrared emissions at 15 μm is the primary radiative cooling mechanism of the thermosphere in the altitude range of 100-135 km. This paper explores the role of two important diurnal nonmigrating tides, the DE2 and DE3, in the modulation of CO2 15 μm emissions during the solar minimum year 2008 by (i) analyzing Sounding the Atmosphere using Broadband Emission Radiometry (SABER) CO2 cooling rate data and (ii) photochemical modeling using dynamical tides from the empirical Climatological Tidal Model of the Thermosphere model. Tidal diagnostics of SABER data shows that the CO2 cooling rate amplitudes for the DE2 and DE3 components are on the order of approximately 20-50% relative to the monthly means, and they maximize around the lower bound (100 km) of the analyzed height interval. The photochemical modeling reproduces the observed results, albeit with systematic amplitude differences which is likely related to the uncertainty in the model input backgrounds, especially atomic oxygen. The main tidal coupling mechanism is found to be the temperature dependence of the collisional excitation of the CO2 ν2 vibrational state. However, neutral density becomes equally important above ˜110 km, thereby explaining observed evanescent DE2 and DE3 phases which are not present in temperature tides. The contribution of vertical tidal advection is comparatively small. The relative importance of the coupling mechanisms is the same at all latitudes/seasons. These results indicate that upward propagating nonmigrating tides forced by latent heat release in the lower atmosphere impact the thermospheric energy budget by modulating the longitudinal/local time behavior of the CO2 infrared cooling.

High-resolution modelling of atmospheric dispersion of dense gas using TWODEE-2.1: application to the 1986 Lake Nyos limnic eruption

NASA Astrophysics Data System (ADS)

Folch, Arnau; Barcons, Jordi; Kozono, Tomofumi; Costa, Antonio

2017-06-01

Atmospheric dispersal of a gas denser than air can threat the environment and surrounding communities if the terrain and meteorological conditions favour its accumulation in topographic depressions, thereby reaching toxic concentration levels. Numerical modelling of atmospheric gas dispersion constitutes a useful tool for gas hazard assessment studies, essential for planning risk mitigation actions. In complex terrains, microscale winds and local orographic features can have a strong influence on the gas cloud behaviour, potentially leading to inaccurate results if not captured by coarser-scale modelling. We introduce a methodology for microscale wind field characterisation based on transfer functions that couple a mesoscale numerical weather prediction model with a microscale computational fluid dynamics (CFD) model for the atmospheric boundary layer. The resulting time-dependent high-resolution microscale wind field is used as input for a shallow-layer gas dispersal model (TWODEE-2.1) to simulate the time evolution of CO2 gas concentration at different heights above the terrain. The strategy is applied to review simulations of the 1986 Lake Nyos event in Cameroon, where a huge CO2 cloud released by a limnic eruption spread downslopes from the lake, suffocating thousands of people and animals across the Nyos and adjacent secondary valleys. Besides several new features introduced in the new version of the gas dispersal code (TWODEE-2.1), we have also implemented a novel impact criterion based on the percentage of human fatalities depending on CO2 concentration and exposure time. New model results are quantitatively validated using the reported percentage of fatalities at several locations. The comparison with previous simulations that assumed coarser-scale steady winds and topography illustrates the importance of high-resolution modelling in complex terrains.

Endocannabinoid Release Modulates Electrical Coupling between CCK Cells Connected via Chemical and Electrical Synapses in CA1

PubMed Central

Iball, Jonathan; Ali, Afia B.

2011-01-01

Electrical coupling between some subclasses of interneurons is thought to promote coordinated firing that generates rhythmic synchronous activity in cortical regions. Synaptic activity of cholecystokinin (CCK) interneurons which co-express cannabinoid type-1 (CB1) receptors are powerful modulators of network activity via the actions of endocannabinoids. We investigated the modulatory actions of endocannabinoids between chemically and electrically connected synapses of CCK cells using paired whole-cell recordings combined with biocytin and double immunofluorescence labeling in acute slices of rat hippocampus at P18–20 days. CA1 stratum radiatum CCK Schaffer collateral-associated cells were coupled electrically with each other as well as CCK basket cells and CCK cells with axonal projections expanding to dentate gyrus. Approximately 50% of electrically coupled cells received facilitating, asynchronously released inhibitory postsynaptic potential (IPSPs) that curtailed the steady-state coupling coefficient by 57%. Tonic CB1 receptor activity which reduces inhibition enhanced electrical coupling between cells that were connected via chemical and electrical synapses. Blocking CB1 receptors with antagonist, AM-251 (5 μM) resulted in the synchronized release of larger IPSPs and this enhanced inhibition further reduced the steady-state coupling coefficient by 85%. Depolarization induced suppression of inhibition (DSI), maintained the asynchronicity of IPSP latency, but reduced IPSP amplitudes by 95% and enhanced the steady-state coupling coefficient by 104% and IPSP duration by 200%. However, DSI did not did not enhance electrical coupling at purely electrical synapses. These data suggest that different morphological subclasses of CCK interneurons are interconnected via gap junctions. The synergy between the chemical and electrical coupling between CCK cells probably plays a role in activity-dependent endocannabinoid modulation of rhythmic synchronization. PMID:22125513

Field validation of a free-agent cellular automata model of fire spread with fire–atmosphere coupling

Treesearch

Gary Achtemeier

2012-01-01

A cellular automata fire model represents ‘elements’ of fire by autonomous agents. A few simple algebraic expressions substituted for complex physical and meteorological processes and solved iteratively yield simulations for ‘super-diffusive’ fire spread and coupled surface-layer (2-m) fire–atmosphere processes. Pressure anomalies, which are integrals of the thermal...

A Numerical Study of Tropical Sea-Air Interactions Using a Cloud Resolving Model Coupled with an Ocean Mixed-Layer Model

NASA Technical Reports Server (NTRS)

Shie, Chung-Lin; Tao, Wei-Kuo; Johnson, Dan; Simpson, Joanne; Li, Xiaofan; Sui, Chung-Hsiung; Einaudi, Franco (Technical Monitor)

2001-01-01

Coupling a cloud resolving model (CRM) with an ocean mixed layer (OML) model can provide a powerful tool for better understanding impacts of atmospheric precipitation on sea surface temperature (SST) and salinity. The objective of this study is twofold. First, by using the three dimensional (3-D) CRM-simulated (the Goddard Cumulus Ensemble model, GCE) diabatic source terms, radiation (longwave and shortwave), surface fluxes (sensible and latent heat, and wind stress), and precipitation as input for the OML model, the respective impact of individual component on upper ocean heat and salt budgets are investigated. Secondly, a two-way air-sea interaction between tropical atmospheric climates (involving atmospheric radiative-convective processes) and upper ocean boundary layer is also examined using a coupled two dimensional (2-D) GCE and OML model. Results presented here, however, only involve the first aspect. Complete results will be presented at the conference.

Using the Model Coupling Toolkit to couple earth system models

USGS Publications Warehouse

Warner, J.C.; Perlin, N.; Skyllingstad, E.D.

2008-01-01

Continued advances in computational resources are providing the opportunity to operate more sophisticated numerical models. Additionally, there is an increasing demand for multidisciplinary studies that include interactions between different physical processes. Therefore there is a strong desire to develop coupled modeling systems that utilize existing models and allow efficient data exchange and model control. The basic system would entail model "1" running on "M" processors and model "2" running on "N" processors, with efficient exchange of model fields at predetermined synchronization intervals. Here we demonstrate two coupled systems: the coupling of the ocean circulation model Regional Ocean Modeling System (ROMS) to the surface wave model Simulating WAves Nearshore (SWAN), and the coupling of ROMS to the atmospheric model Coupled Ocean Atmosphere Prediction System (COAMPS). Both coupled systems use the Model Coupling Toolkit (MCT) as a mechanism for operation control and inter-model distributed memory transfer of model variables. In this paper we describe requirements and other options for model coupling, explain the MCT library, ROMS, SWAN and COAMPS models, methods for grid decomposition and sparse matrix interpolation, and provide an example from each coupled system. Methods presented in this paper are clearly applicable for coupling of other types of models. ?? 2008 Elsevier Ltd. All rights reserved.

Stimulation of microbial nitrogen cycling in aquatic ecosystems by benthic macrofauna: mechanisms and environmental implications

NASA Astrophysics Data System (ADS)

Stief, P.

2013-12-01

Invertebrate animals that live at the bottom of aquatic ecosystems (i.e., benthic macrofauna) are important mediators between nutrients in the water column and microbes in the benthos. The presence of benthic macrofauna stimulates microbial nutrient dynamics through different types of animal-microbe interactions, which potentially affect the trophic status of aquatic ecosystems. This review contrasts three types of animal-microbe interactions in the benthos of aquatic ecosystems: (i) ecosystem engineering, (ii) grazing, and (iii) symbiosis. Their specific contributions to the turnover of fixed nitrogen (mainly nitrate and ammonium) and the emission of the greenhouse gas nitrous oxide are evaluated. Published data indicate that ecosystem engineering by sediment-burrowing macrofauna stimulates benthic nitrification and denitrification, which together allows fixed nitrogen removal. However, the release of ammonium from sediments is enhanced more strongly than the sedimentary uptake of nitrate. Ecosystem engineering by reef-building macrofauna increases nitrogen retention and ammonium concentrations in shallow aquatic ecosystems, but allows organic nitrogen removal through harvesting. Grazing by macrofauna on benthic microbes apparently has small or neutral effects on nitrogen cycling. Animal-microbe symbioses provide abundant and distinct benthic compartments for a multitude of nitrogen-cycle pathways. Recent studies reveal that ecosystem engineering, grazing, and symbioses of benthic macrofauna significantly enhance nitrous oxide emission from shallow aquatic ecosystems. The beneficial effect of benthic macrofauna on fixed nitrogen removal through coupled nitrification-denitrification can thus be offset by the concurrent release of (i) ammonium that stimulates aquatic primary production and (ii) nitrous oxide that contributes to global warming. Overall, benthic macrofauna intensifies the coupling between benthos, pelagial, and atmosphere through enhanced turnover and transport of nitrogen.

Stimulation of microbial nitrogen cycling in aquatic ecosystems by benthic macrofauna: mechanisms and environmental implications

NASA Astrophysics Data System (ADS)

Stief, P.

2013-07-01

Invertebrate animals that live at the bottom of aquatic ecosystems (i.e., benthic macrofauna) are important mediators between nutrients in the water column and microbes in the benthos. The presence of benthic macrofauna stimulates microbial nutrient dynamics through different types of animal-microbe interactions, which potentially affect the trophic status of aquatic ecosystems. This review contrasts three types of animal-microbe interactions in the benthos of aquatic ecosystems: (i) ecosystem engineering, (ii) grazing, and (iii) symbiosis. Their specific contributions to the turnover of fixed nitrogen (mainly nitrate and ammonium) and the emission of the greenhouse gas nitrous oxide are evaluated. Published data indicate that ecosystem engineering by sediment-burrowing macrofauna stimulates benthic nitrification and denitrification, which together allows fixed nitrogen removal. However, the release of ammonium from sediments often is enhanced even more than the sedimentary uptake of nitrate. Ecosystem engineering by reef-building macrofauna increases nitrogen retention and ammonium concentrations in shallow aquatic ecosystems, but allows organic nitrogen removal through harvesting. Grazing by macrofauna on benthic microbes apparently has small or neutral effects on nitrogen cycling. Animal-microbe symbioses provide abundant and distinct benthic compartments for a multitude of nitrogen-cycle pathways. Recent studies revealed that ecosystem engineering, grazing, and symbioses of benthic macrofauna significantly enhance nitrous oxide emission from shallow aquatic ecosystems. The beneficial effect of benthic macrofauna on fixed nitrogen removal through coupled nitrification-denitrification can thus be offset by the concurrent release of (i) ammonium that stimulates aquatic primary production and (ii) nitrous oxide that contributes to global warming. Overall, benthic macrofauna intensifies the coupling between benthos, pelagial, and atmosphere through enhanced turnover and transport of nitrogen.

Coupled atmosphere-ocean models of Titan's past

NASA Technical Reports Server (NTRS)

Mckay, Christopher P.; Pollack, James B.; Lunine, Jonathan I.; Courtin, Regis

1993-01-01

The behavior and possible past evolution of fully coupled atmosphere and ocean model of Titan are investigated. It is found that Titan's surface temperature was about 20 K cooler at 4 Gyr ago and will be about 5 K warmer 0.5 Gyr in the future. The change in solar luminosity and the conversion of oceanic CH4 to C2H6 drive the evolution of the ocean and atmosphere over time. Titan appears to have experienced a frozen epoch about 3 Gyr ago independent of whether an ocean is present or not. This finding may have important implications for understanding the inventory of Titan's volatile compounds.

Modes of North Atlantic Decadal Variability in the ECHAM1/LSG Coupled Ocean-Atmosphere General Circulation Model.

NASA Astrophysics Data System (ADS)

Zorita, Eduardo; Frankignoul, Claude

1997-02-01

The climate variability in the North Atlantic sector is investigated in a 325-yr integration of the ECHAM1/ LSG coupled ocean-atmosphere general circulation model. At the interannual timescale, the coupled model behaves realistically and sea surface temperature (SST) anomalies arise as a response of the oceanic surface layer to the stochastic forcing by the atmosphere, with the heat exchanges both generating and damping the SST anomalies. In the ocean interior, the temperature spectra are red up to a period of about 20 years, and substantial decadal fluctuations are found in the upper kilometer or so of the water column. Using extended empirical orthogonal function analysis, two distinct quasi-oscillatory modes of ocean-atmosphere variability are identified, with dominant periods of about 20 and 10 years, respectively. The oceanic changes in both modes reflect the direct forcing by the atmosphere through anomalous air-sea fluxes and Ekman pumping, which after some delay affects the intensity of the subtropical and subpolar gyres. The SST is also strongly modulated by the gyre currents. In the thermocline, the temperature and salinity fluctuations are in phase, as if caused by thermocline displacements, and they have no apparent connection with the thermohaline circulation. The 20-yr mode is the most energetic one; it is easily seen in the thermocline and can be found in SST data, but it is not detected in the atmosphere alone. As there is no evidence of positive ocean-atmosphere feedback, the 20-yr mode primarily reflects the passive response of the ocean to atmospheric fluctuations, which may be in part associated with climate anomalies appearing a few years earlier in the North Pacific. The 10-yr mode is more surface trapped in the ocean. Although the mode is most easily seen in the temperature variations of the upper few hundred meters of the ocean, it is also detected in the atmosphere alone and thus appears to be a coupled ocean-atmosphere mode. In both modes, the surface heat flux acts neutrally on the associated SST anomalies once they have been generated, so that their persistence appears to be due in part to an overall adjustment of the air-sea heat exchanges to the SST patterns.

Diagnosing the Nature of Land-Atmosphere Coupling During the 2006-7 Dry/Wet Extremes in the U. S. Southern Great Plains

NASA Technical Reports Server (NTRS)

Santanello, Joseph A.; Peters-Lidard, Christa D.; Kennedy, Aaron D.; Kumar, Sujay; Dong, Xiquan

2011-01-01

Land-atmosphere (L-A) interactions play a critical role in determining the diurnal evolution of land surface and planetary boundary layer (PBL) temperature and moisture states and fluxes. In turn, these interactions regulate the strength of the connection between surface moisture and precipitation in a coupled system. To address deficiencies in numerical weather prediction and climate models due to improper treatment of L-A interactions, recent studies have focused on development of diagnostics to quantify the strength and accuracy of the land-PBL coupling at the process-level. In this study, a diagnosis of the nature and impacts of local land-atmosphere coupling (LoCo) during dry and wet extreme conditions is presented using a combination of models and observations during the summers of2006-7 in the U.S. Southern Great Plains. Specifically, the Weather Research and Forecasting (WRF) model has been coupled to NASA's Land Information System (LIS), which provides a flexible and high resolution representation and initialization of land surface physics and states. A range of diagnostics exploring the links and feedbacks between soil moisture and precipitation are examined for the dry/wet regimes of this region, along with the behavior and accuracy of different land-PBL scheme couplings under these conditions. Results demonstrate how LoCo diagnostics can be applied to coupled model components in the context of their integrated impacts on the process-chain connecting the land surface to the PBL and support of hydrological anomalies.

The role of evapotranspiration fluxes in summertime precipitation in Central Europe: coupled groundwater-atmosphere simulations with the WRF-LEAFHYDRO system.

NASA Astrophysics Data System (ADS)

Regueiro Sanfiz, Sabela; Gómez, Breo; Miguez Macho, Gonzalo

2017-04-01

Because of its continental position, Central Europe summertime rainfall is largely dependent on local or regional dynamics, with precipitation water possibly also significantly dependent on local sources. We investigate here land-atmosphere feedbacks over inland Europe focusing in particular on evapotranspiration-soil moisture connections and precipitation recycling ratios. For this purpose, a set of simulations were performed with the Weather Research and Forecasting (WRF) model coupled to LEAFHYDRO soil-vegetation-hydrology model. The LEAFHYDRO Land Surface Model includes a groundwater parameterization with a dynamic water table fully coupling groundwater to the soil-vegetation and surface waters via two-way fluxes. A water tagging capability in the WRF model is used to quantify evapotranspiration contribution to precipitation over the region. Several years are considered, including summertime 2002, during which severe flooding occurred. Preliminary results from our simulations highlight the link of large areas with shallow water with high air moisture values through the summer season; and the importance of the contribution of evapotranspiration to summertime precipitation. Consequently, results show the advantages of using a fully coupled hydrology-atmospheric modeling system.

DOD Pico-Satellite known as ANDE released from the STS-116 shuttle payload bay

NASA Image and Video Library

2006-12-21

S116-E-07837 (21 Dec. 2006) --- As seen through windows on the aft flight deck of Space Shuttle Discovery, a Department of Defense pico-satellite known as Atmospheric Neutral Density Experiment (ANDE) is released from the shuttle's payload bay by STS-116 crewmembers. ANDE consists of two micro-satellites which will measure the density and composition of the low Earth orbit (LEO) atmosphere while being tracked from the ground. The data will be used to better predict the movement of objects in orbit.

DOD Pico-Satellite known as ANDE released from the STS-116 shuttle payload bay

NASA Image and Video Library

2006-12-21

S116-E-07831 (21 Dec. 2006) --- As seen through windows on the aft flight deck of Space Shuttle Discovery, a Department of Defense pico-satellite known as Atmospheric Neutral Density Experiment (ANDE) is released from the shuttle's payload bay by STS-116 crewmembers. ANDE consists of two micro-satellites which will measure the density and composition of the low Earth orbit (LEO) atmosphere while being tracked from the ground. The data will be used to better predict the movement of objects in orbit.

DOD Pico-Satellite known as ANDE released from the STS-116 shuttle payload bay

NASA Image and Video Library

2006-12-21

S116-E-07838 (21 Dec. 2006) --- As seen through windows on the aft flight deck of Space Shuttle Discovery, a Department of Defense pico-satellite known as Atmospheric Neutral Density Experiment (ANDE) is released from the shuttle's payload bay by STS-116 crewmembers. ANDE consists of two micro-satellites which will measure the density and composition of the low Earth orbit (LEO) atmosphere while being tracked from the ground. The data will be used to better predict the movement of objects in orbit.

Late Veneer consequences on Venus' long term evolution

NASA Astrophysics Data System (ADS)

Gillmann, C.; Golabek, G.; Tackley, P. J.; Raymond, S. N.

2017-12-01

Modelling of Venus' evolution is able to produce scenarios consistent with present-day observation. These results are however heavily dependent on atmosphere escape and initial volatile inventory. This primordial history (the first 500 Myr) is heavily influenced by collisions. We investigate how Late Veneer impacts change the initial state of Venus and their consequences on its coupled mantle/atmosphere evolution. We focus on volatile fluxes: atmospheric escape and mantle degassing. Mantle dynamics is simulated using the StagYY code. Atmosphere escape covers both thermal and non-thermal processes. Surface conditions are calculated with a radiative-convective model. Feedback of the atmosphere on the mantle through surface temperature is included. Large impacts are capable of contributing to atmospheric escape, volatile replenishment and energy transfer. We use the SOVA hydrocode to take into account volatile loss and deposition during a collision. Large impacts are not numerous enough to substantially erode Venus' atmosphere. Single impacts don't have enough eroding power. Swarms of small bodies (<50km radius) might be a better candidate for this process. The amount of volatiles brought by large ordinary chondrite impactors is superior to losses and comparable to the degassing caused by the impact. Carbonaceous chondrite impactors are unlikely: they release too many volatiles, causing surface temperature to stay above 900K up to present-day. Mantle dynamics can also be modified by the heating caused by impacts. Heated material propagates by spreading across the upper mantle due to its buoyancy. Old crust is destroyed or remixed in the mantle. A large part of the upper mantle melts, leading to its depletion and degassing. With enough evenly distributed high energy impacts, the mantle can be depleted by more than 90% of its volatiles during Late Veneer. This drastically cuts down degassing in the late history of the planet and leads to lower present-day surface temperatures. Total depletion of the mantle seems unlikely, meaning either few large impacts (1 to 4) or low energy (slow, grazing…) collisions. Combined with the lack of plate tectonics and volatile recycling in the interior of Venus, Late Veneer collisions could help explain why Venus seems dry today.

PROBABILISTIC CHARACTERIZATION OF ATMOSPHERIC TRANSPORT AND DISPERSION

EPA Science Inventory

Dispersion models are used to assess the possible extent and severity of accidental or terrorist releases of toxic materials. Most operational models only provide a characterization of average concentrations and conditions following a release. Knowledge of the variability about...

Advective removal of intraparticle uranium from contaminated vadose zone sediments, Hanford, U.S.

PubMed

Ilton, Eugene S; Qafoku, Nikolla P; Liu, Chongxuan; Moore, Dean A; Zachara, John M

2008-03-01

A column study on U(VI)-contaminated vadose zone sediments from the Hanford Site, WA, was performed to investigate U(VI) release kinetics with water advection and variable geochemical conditions. The sediments were collected from an area adjacent to and below tank BX-102 that was contaminated as a result of a radioactive tank waste overfill event. The primary reservoir for U(VI) in the sediments are micrometer-size precipitates composed of nanocrystallite aggregates of a Na-U-Silicate phase, most likely Na-boltwoodite, that nucleated and grew within microfractures of the plagioclase component of sand-sized granitic clasts. Two sediment samples, with different U(VI) concentrations and intraparticle mass transfer properties, were leached with advective flows of three different solutions. The influent solutions were all calcite-saturated and in equilibrium with atmospheric CO2. One solution was prepared from DI water, the second was a synthetic groundwater (SGW) with elevated Na that mimicked groundwater at the Hanford site, and the third was the same SGW but with both elevated Na and Si. The latter two solutions were employed, in part, to test the effect of saturation state on U(VI) release. For both sediments, and all three electrolytes, there was an initial rapid release of U(VI) to the advecting solution followed by slower near steady-state release. U(VI)aq concentrations increased during subsequent stop-flow events. The electrolytes with elevated Na and Si depressed U(VL)aq concentrations in effluent solutions. Effluent U(VI)aq concentrations for both sediments and all three electrolytes were simulated reasonably well by a three domain model (the advecting fluid, fractures, and matrix) that coupled U(VI) dissolution, intraparticle U(VI)aq diffusion, and interparticle advection, where diffusion and dissolution properties were parameterized in a previous batch study.

Hydraulic Pressure during Fluid Flow Regulates Purinergic Signaling and Cytoskeleton Organization of Osteoblasts.

PubMed

Gardinier, Joseph D; Gangadharan, Vimal; Wang, Liyun; Duncan, Randall L

2014-06-01

During physiological activities, osteoblasts experience a variety of mechanical forces that stimulate anabolic responses at the cellular level necessary for the formation of new bone. Previous studies have primarily investigated the osteoblastic response to individual forms of mechanical stimuli. However in this study, we evaluated the response of osteoblasts to two simultaneous, but independently controlled stimuli; fluid flow-induced shear stress (FSS) and static or cyclic hydrostatic pressure (SHP or CHP, respectively). MC3T3-E1 osteoblasts-like cells were subjected to 12dyn/cm 2 FSS along with SHP or CHP of varying magnitudes to determine if pressure enhances the anabolic response of osteoblasts during FSS. For both SHP and CHP, the magnitude of hydraulic pressure that induced the greatest release of ATP during FSS was 15 mmHg. Increasing the hydraulic pressure to 50 mmHg or 100 mmHg during FSS attenuated the ATP release compared to 15 mmHg during FSS. Decreasing the magnitude of pressure during FSS to atmospheric pressure reduced ATP release to that of basal ATP release from static cells and inhibited actin reorganization into stress fibers that normally occurred during FSS with 15 mmHg of pressure. In contrast, translocation of nuclear factor kappa B (NFκB) to the nucleus was independent of the magnitude of hydraulic pressure and was found to be mediated through the activation of phospholipase-C (PLC), but not src kinase. In conclusion, hydraulic pressure during FSS was found to regulate purinergic signaling and actin cytoskeleton reorganization in the osteoblasts in a biphasic manner, while FSS alone appeared to stimulate NFκB translocation. Understanding the effects of hydraulic pressure on the anabolic responses of osteoblasts during FSS may provide much needed insights into the physiologic effects of coupled mechanical stimuli on osteogenesis.

Hydraulic Pressure during Fluid Flow Regulates Purinergic Signaling and Cytoskeleton Organization of Osteoblasts

PubMed Central

Gardinier, Joseph D.; Gangadharan, Vimal; Wang, Liyun; Duncan, Randall L.

2014-01-01

During physiological activities, osteoblasts experience a variety of mechanical forces that stimulate anabolic responses at the cellular level necessary for the formation of new bone. Previous studies have primarily investigated the osteoblastic response to individual forms of mechanical stimuli. However in this study, we evaluated the response of osteoblasts to two simultaneous, but independently controlled stimuli; fluid flow-induced shear stress (FSS) and static or cyclic hydrostatic pressure (SHP or CHP, respectively). MC3T3-E1 osteoblasts-like cells were subjected to 12dyn/cm2 FSS along with SHP or CHP of varying magnitudes to determine if pressure enhances the anabolic response of osteoblasts during FSS. For both SHP and CHP, the magnitude of hydraulic pressure that induced the greatest release of ATP during FSS was 15 mmHg. Increasing the hydraulic pressure to 50 mmHg or 100 mmHg during FSS attenuated the ATP release compared to 15 mmHg during FSS. Decreasing the magnitude of pressure during FSS to atmospheric pressure reduced ATP release to that of basal ATP release from static cells and inhibited actin reorganization into stress fibers that normally occurred during FSS with 15 mmHg of pressure. In contrast, translocation of nuclear factor kappa B (NFκB) to the nucleus was independent of the magnitude of hydraulic pressure and was found to be mediated through the activation of phospholipase-C (PLC), but not src kinase. In conclusion, hydraulic pressure during FSS was found to regulate purinergic signaling and actin cytoskeleton reorganization in the osteoblasts in a biphasic manner, while FSS alone appeared to stimulate NFκB translocation. Understanding the effects of hydraulic pressure on the anabolic responses of osteoblasts during FSS may provide much needed insights into the physiologic effects of coupled mechanical stimuli on osteogenesis. PMID:24910719

Role of Earth's plasmasphere in coupling of upper atmosphere

NASA Astrophysics Data System (ADS)

Singh, A. K.; Mishra, Sandhya; Dohare, S. K.

2010-02-01

The near-Earth space environment is a complex, ever changing system of magnetized plasmas whose behaviour has a profound impact upon our technology dependent society. The exploration of the cold, relatively dense, inner region of upper atmosphere (the plasmasphere) and its unexpectedly sharp outer boundary (the plasma pause) has proceeded through a combination of in-situ observations and ground based whistler observations. Studies have shown that plasmasphere is highly variable both spatially and temporally responding to changes in geomagnetic indices, ring current, penetration and shielding electric fields and subauroral electric fields. Consequently the plasmasphere exhibits erosion, emptying and refilling during active times. Infact, it is the electric field that plays one of the most important roles in coupling of upper atmosphere. The atmospheric dynamo is the main generator of the large-scale electric field in the upper atmosphere. It arises because of a special situation which electrons and ions move with different velocities across the magnetic field because of different collisions between electrons and neutral particles and ions with neutral particles. This process leads to charge separation and consequently to an electric field. In the present paper, storm/ quiet period VLF whistler data recorded at lower latitudes/mid latitudes are analyzed and attempt has been made to look at plasmasphere response on coupling of ionosphere and magnetosphere.

D/H in Water Evolved from Martian Rocks in Gale Crater

NASA Astrophysics Data System (ADS)

Mahaffy, P. R.; Franz, H. B.; Atreya, S. K.; Webster, C. R.

2017-12-01

The Sample Analysis at Mars (SAM) instrument suite with its Quadrupole Mass Spectrometer (QMS) and Tunable Laser Spectrometer (TSL) measures isotopes such as δ34S in SO2 [1], δ37Cl in HCl [2], δ15N in N2 or NO [3], δ13C in CH4 [4], δ13C and δ18O in CO2 [5-6], δD in H2O [7], and a variety of noble gas isotopes [8-9]. Fractionation of isotopes of H, C, O, N, Ar, and Xe indicates a substantial loss of atmosphere to space. For xenon this may have occurred early in the history of Mars by hydrodynamic escape [10] or spread over time for C, O, N, and Ar [11]. Nevertheless, the detailed history of atmospheric loss and the predictions of the climate when the Gale crater was a lake are still not well constrained. Isotopes from light elements that are presently measured in the atmosphere but that were also locked into minerals in rocks more than 3 billion years ago are of particular interest as they may provide additional constraints on the history of atmospheric loss. These include 15N/14N presently measured in atmospheric N2 [3] but also in nitrogen released from ancient nitrates as NO [12] and D/H in atmospheric water [13] and in water or hydroxyl locked into minerals and released in the SAM evolved gas analysis (EGA) experiments [7]. D/H in water can be measured by both the TSL and the QMS. Typically the D/H decreases over the course of the EGA temperature ramp, since gas that has exchanged with the current atmosphere is released at lower temperatures. Less easily exchanged gas reflecting the D/H ratio in the water of formation of a mineral, such as that from the dehydroxylation of a phylosillicate, is released at higher temperatures. We will examine some of the D/H measurements made on drilled and powdered rocks and the trends in the variation of the D/H ratio with release temperature. We will compare these ratios with the D/H in atmospheric water and discuss possible consequences for loss of D/H over time. References: [1] Franz et al., in press. [2] Farley et al. (2016) EPSL 438. [3] Wong et al. (2013) GRL 40. [4] Webster et al. (2011) PSS 59. [5] Mahaffy et al. (2013) Science 341. [6] Webster et al. (2013) Science 341. [7] Mahaffy et al. (2015) Science 347. [8] Atreya et al. (2013) GRL 40. [9] Conrad et al. (2016) EPSL 454. [10] Pepin et al. (2006) EPSL 252. [11] Jakosky et al. (1994) Icarus 111. [12] Stern, this meeting. [13] Villaneuva et al. (2015) Science 348.

COUPLING

DOEpatents

Hawke, B.C.

1963-02-26

This patent relates to a releasable coupling connecting a control rod to a control rod drive. This remotely operable coupling mechanism can connect two elements which are laterally and angviarly misaligned, and provides a means for sensing the locked condition of the elements. The coupling utilizes a spherical bayonet joint which is locked against rotation by a ball detent lock. (AEC)

Snow-atmosphere coupling and its impact on temperature variability and extremes over North America

NASA Astrophysics Data System (ADS)

Diro, G. T.; Sushama, L.; Huziy, O.

2018-04-01

The impact of snow-atmosphere coupling on climate variability and extremes over North America is investigated using modeling experiments with the fifth generation Canadian Regional Climate Model (CRCM5). To this end, two CRCM5 simulations driven by ERA-Interim reanalysis for the 1981-2010 period are performed, where snow cover and depth are prescribed (uncoupled) in one simulation while they evolve interactively (coupled) during model integration in the second one. Results indicate systematic influence of snow cover and snow depth variability on the inter-annual variability of soil and air temperatures during winter and spring seasons. Inter-annual variability of air temperature is larger in the coupled simulation, with snow cover and depth variability accounting for 40-60% of winter temperature variability over the Mid-west, Northern Great Plains and over the Canadian Prairies. The contribution of snow variability reaches even more than 70% during spring and the regions of high snow-temperature coupling extend north of the boreal forests. The dominant process contributing to the snow-atmosphere coupling is the albedo effect in winter, while the hydrological effect controls the coupling in spring. Snow cover/depth variability at different locations is also found to affect extremes. For instance, variability of cold-spell characteristics is sensitive to snow cover/depth variation over the Mid-west and Northern Great Plains, whereas, warm-spell variability is sensitive to snow variation primarily in regions with climatologically extensive snow cover such as northeast Canada and the Rockies. Furthermore, snow-atmosphere interactions appear to have contributed to enhancing the number of cold spell days during the 2002 spring, which is the coldest recorded during the study period, by over 50%, over western North America. Additional results also provide useful information on the importance of the interactions of snow with large-scale mode of variability in modulating temperature extreme characteristics.

Control of the neurovascular coupling by nitric oxide-dependent regulation of astrocytic Ca2+ signaling

PubMed Central

Muñoz, Manuel F.; Puebla, Mariela; Figueroa, Xavier F.

2015-01-01

Neuronal activity must be tightly coordinated with blood flow to keep proper brain function, which is achieved by a mechanism known as neurovascular coupling. Then, an increase in synaptic activity leads to a dilation of local parenchymal arterioles that matches the enhanced metabolic demand. Neurovascular coupling is orchestrated by astrocytes. These glial cells are located between neurons and the microvasculature, with the astrocytic endfeet ensheathing the vessels, which allows fine intercellular communication. The neurotransmitters released during neuronal activity reach astrocytic receptors and trigger a Ca2+ signaling that propagates to the endfeet, activating the release of vasoactive factors and arteriolar dilation. The astrocyte Ca2+ signaling is coordinated by gap junction channels and hemichannels formed by connexins (Cx43 and Cx30) and channels formed by pannexins (Panx-1). The neuronal activity-initiated Ca2+ waves are propagated among neighboring astrocytes directly via gap junctions or through ATP release via connexin hemichannels or pannexin channels. In addition, Ca2+ entry via connexin hemichannels or pannexin channels may participate in the regulation of the astrocyte signaling-mediated neurovascular coupling. Interestingly, nitric oxide (NO) can activate connexin hemichannel by S-nitrosylation and the Ca2+-dependent NO-synthesizing enzymes endothelial NO synthase (eNOS) and neuronal NOS (nNOS) are expressed in astrocytes. Therefore, the astrocytic Ca2+ signaling triggered in neurovascular coupling may activate NO production, which, in turn, may lead to Ca2+ influx through hemichannel activation. Furthermore, NO release from the hemichannels located at astrocytic endfeet may contribute to the vasodilation of parenchymal arterioles. In this review, we discuss the mechanisms involved in the regulation of the astrocytic Ca2+ signaling that mediates neurovascular coupling, with a special emphasis in the possible participation of NO in this process. PMID:25805969

Seismic Correlation and Coupling from Underground, Surface, to the Ionosphere

NASA Astrophysics Data System (ADS)

Wang, J. S.; Waysand, G.

2009-12-01

Electromagnetic activity correlated to seismicity is displayed in a variety of ways. Earthquake precursors and aftershocks associated with local fault slips have been detected regionally by visual observations and radar reflections, and globally by satellite measurements of electromagnetic profiles. Magnetic excitations have recently been measured underground that associated with major earthquakes (e.g., the 2008 Sichuan and the 2006 Pingtung earthquakes). In all cases, the frequencies are extremely low; hence, the corresponding wavelengths are extremely large. In other term, wherever an earthquake occurs on Earth, any electromagnetic measurement of it is always near-field from the signal source. Thus, signal-to-noise ratio is the only limiting factor. The increasing abundance of observations, and the variety of instruments enabling these observations, requires investigators to look beyond borders of their individual discipline and adopt a global approach to the problem. To elucidate the dynamic generation and propagation of seismic-induced electromagnetic signals, it is important to assess from small to large scales the variability of (1) the seismic-electromagnetic coupling at localized zones and block boundaries, (2) the potential signal paths through the earth geomagnetic fields, and (3) the ionosphere and atmospheric measurements and observations. The pre-earthquake signals as potential precursors have generated great interests for decades, especially with the deployments of satellites for geophysical measurements. The emerging understanding is that stress buildups and releases induce electromagnetic emissions which are likely associated with charged particle movements, propagations mainly along waveguides through the earth magnetic field to the atmosphere and ionosphere. The globally distributed perturbations and profiles above ground are systematically mapped. The signals could also be transmitted nearly vertically from epicenters to the ground and beyond, especially for post-earthquake periods with displacements associated with seismic wave arrivals at the ground surfaces. We assess the correlation and coupling among signals measured at depths, on the surface, and in the sky. While the main focus is on electromagnetic signals associated with earthquakes, there are many relevant measurements and analyses among seismic, rock mechanical, hydrochemical, electromagnetic, atmospheric, ionospheric and other processes and phenomena. The correlation of different signals in space and time can elucidate the different coupling and channeling of signals. The demonstrated low noise advantage of underground seismic-magnetic detections of global signals at the Laboratoire Souterrain Bas Bruit de Rustrel-Pays d'Apt should set the example for the establishment of equivalent stations worldwide in other underground research laboratories. We emphasize the adoption of international and inter-disciplinary approaches that can contribute to better understanding of mechanisms among different earthquake and tectonic forces, and lead to improved assessment of earthquake and related natural hazards.

Role of upper-ocean on the intensity of Bay of Bengal cyclone `Phailin' as revealed by coupled simulation using Mesoscale Coupled Modeling System (WRF-ROMS)

NASA Astrophysics Data System (ADS)

Mani, B.; Mandal, M.

2016-12-01

Numerical prediction of tropical cyclone (TC) track has improved significantly in recent years, but not the intensity. It is well accepted that TC induced sea surface temperature (SST) cooling in conjunction with pre-existing upper-ocean features have major influences on tropical cyclone intensity. Absence of two-way atmosphere-ocean feedback in the stand-alone atmosphere models has major consequences on their prediction of TC intensity. The present study investigates the role of upper-ocean on prediction of TC intensity and track based on coupled and uncoupled simulation of the Bay of Bengal (BoB) cyclone `Phailin'. The coupled simulation is conducted with the Mesoscale Coupled Modeling System (MCMS) which is a fully coupled atmosphere-ocean modeling system that includes the non-hydrostatic atmospheric model (WRF-ARW) and the three-dimensional hydrostatic ocean model (ROMS). The uncoupled simulation is performed using the atmosphere component of MCMS i.e., the customized version of WRF-ARW for BoB cyclones with prescribed (RTG) SST. The track and intensity of the storm is significantly better simulated by the MCMS and closely followed the observation. The peak intensity, landfall position and time are accurately predicted by MCMS, whereas the uncoupled simulation over predicted the storm intensity. Validation of storm induced SST cooling with the merged microwave-infrared satellite SST indicates that the MCMS simulation shows better correlation both in terms of spatial spread of cold wake and its magnitude. The analysis also suggests that the Pre-existing Cyclonic Eddy (PCE) observed adjacent to the storm enhanced the TC induced SST cooling. It is observed that the response of SST (i.e., cooling) to storm intensity is 12hr with 95% statistical significance. The air-sea enthalpy flux shows a clear asymmetry between Front Left (FL) and Rear Right (RR) regime to the storm center where TC induced cooling is more than 0.5K/24hr. The analysis of atmospheric boundary layer reveals the formation of persistent stable boundary layer (SBL) over the cold wake, which caused asymmetry in TC structure by quelling convection in the rainbands downstream to the cold wake. The present study signifies the importance of using MCMS in prediction of the BoB cyclone and encourages further investigation with more cyclone cases.

The South Asian Monsoon and the Tropospheric Biennial Oscillation.

NASA Astrophysics Data System (ADS)

Meehl, Gerald A.

1997-08-01

A mechanism is described that involves the south Asian monsoon as an active part of the tropospheric biennial oscillation (TBO) described in previous studies. This mechanism depends on coupled land-atmosphere-ocean interactions in the Indian sector, large-scale atmospheric east-west circulations in the Tropics, convective heating anomalies over Africa and the Pacific, and tropical-midlatitude interactions in the Northern Hemisphere. A key element for the monsoon role in the TBO is land-sea or meridional tropospheric temperature contrast, with area-averaged surface temperature anomalies over south Asia that are able to persist on a 1-yr timescale without the heat storage characteristics that contribute to this memory mechanism in the ocean. Results from a global coupled general circulation model show that soil moisture anomalies contribute to land-surface temperature anomalies (through latent heat flux anomalies) for only one season after the summer monsoon. A global atmospheric GCM in perpetual January mode is run with observed SSTs with specified convective heating anomalies to demonstrate that convective heating anomalies elsewhere in the Tropics associated with the coupled ocean-atmosphere biennial mechanism can contribute to altering seasonal midlatitude circulation. These changes in the midlatitude longwave pattern, forced by a combination of tropical convective heating anomalies over East Africa, Southeast Asia, and the western Pacific (in association with SST anomalies), are then able to maintain temperature anomalies over south Asia via advection through winter and spring to set up the land-sea meridional tropospheric temperature contrast for the subsequent monsoon. The role of the Indian Ocean, then, is to provide a moisture source and a low-amplitude coupled response component for meridional temperature contrast to help drive the south Asian monsoon. The role of the Pacific is to produce shifts in regionally coupled convection-SST anomalies. These regions are tied together and mutually interact via the large-scale east-west circulation in the atmosphere and contribute to altering midlatitude circulations as well. The coupled model results, and experiments with an atmospheric GCM that includes specified convective heating anomalies, suggest that the influence of south Asian snow cover in the monsoon is not a driving force by itself, but is symptomatic of the larger-scale shift in the midlatitude longwave pattern associated with tropical SST and convective heating anomalies.

Examining Air Quality-Meteorology Interactions on Regional to Hemispheric Scales

EPA Science Inventory

This presentation provides motivation for coupling the atmospheric dynamics and chemistry calculations in air pollution modeling systems, provides an overview of how this coupling is achieved in the WRF-CMAQ 2-way coupled model, presents results from various applications of the m...

Satellite observations of middle atmosphere-thermosphere vertical coupling by gravity waves

NASA Astrophysics Data System (ADS)

Trinh, Quang Thai; Ern, Manfred; Doornbos, Eelco; Preusse, Peter; Riese, Martin

2018-03-01

Atmospheric gravity waves (GWs) are essential for the dynamics of the middle atmosphere. Recent studies have shown that these waves are also important for the thermosphere/ionosphere (T/I) system. Via vertical coupling, GWs can significantly influence the mean state of the T/I system. However, the penetration of GWs into the T/I system is not fully understood in modeling as well as observations. In the current study, we analyze the correlation between GW momentum fluxes observed in the middle atmosphere (30-90 km) and GW-induced perturbations in the T/I. In the middle atmosphere, GW momentum fluxes are derived from temperature observations of the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) satellite instrument. In the T/I, GW-induced perturbations are derived from neutral density measured by instruments on the Gravity field and Ocean Circulation Explorer (GOCE) and CHAllenging Minisatellite Payload (CHAMP) satellites. We find generally positive correlations between horizontal distributions at low altitudes (i.e., below 90 km) and horizontal distributions of GW-induced density fluctuations in the T/I (at 200 km and above). Two coupling mechanisms are likely responsible for these positive correlations: (1) fast GWs generated in the troposphere and lower stratosphere can propagate directly to the T/I and (2) primary GWs with their origins in the lower atmosphere dissipate while propagating upwards and generate secondary GWs, which then penetrate up to the T/I and maintain the spatial patterns of GW distributions in the lower atmosphere. The mountain-wave related hotspot over the Andes and Antarctic Peninsula is found clearly in observations of all instruments used in our analysis. Latitude-longitude variations in the summer midlatitudes are also found in observations of all instruments. These variations and strong positive correlations in the summer midlatitudes suggest that GWs with origins related to convection also propagate up to the T/I. Different processes which likely influence the vertical coupling are GW dissipation, possible generation of secondary GWs, and horizontal propagation of GWs. Limitations of the observations as well as of our research approach are discussed.

CO2 Efflux from Shrimp Ponds in Indonesia

PubMed Central

Sidik, Frida; Lovelock, Catherine E.

2013-01-01

The conversion of mangrove forest to aquaculture ponds has been increasing in recent decades. One of major concerns of this habitat loss is the release of stored ‘blue’ carbon from mangrove soils to the atmosphere. In this study, we assessed carbon dioxide (CO2) efflux from soil in intensive shrimp ponds in Bali, Indonesia. We measured CO2 efflux from the floors and walls of shrimp ponds. Rates of CO2 efflux within shrimp ponds were 4.37 kg CO2 m−2 y−1 from the walls and 1.60 kg CO2 m−2 y−1 from the floors. Combining our findings with published data of aquaculture land use in Indonesia, we estimated that shrimp ponds in this region result in CO2 emissions to the atmosphere between 5.76 and 13.95 Tg y−1. The results indicate that conversion of mangrove forests to aquaculture ponds contributes to greenhouse gas emissions that are comparable to peat forest conversion to other land uses in Indonesia. Higher magnitudes of CO2 emission may be released to atmosphere where ponds are constructed in newly cleared mangrove forests. This study indicates the need for incentives that can meet the target of aquaculture industry without expanding the converted mangrove areas, which will lead to increased CO2 released to atmosphere. PMID:23755306

CO₂ efflux from shrimp ponds in Indonesia.

PubMed

Sidik, Frida; Lovelock, Catherine E

2013-01-01

The conversion of mangrove forest to aquaculture ponds has been increasing in recent decades. One of major concerns of this habitat loss is the release of stored 'blue' carbon from mangrove soils to the atmosphere. In this study, we assessed carbon dioxide (CO₂) efflux from soil in intensive shrimp ponds in Bali, Indonesia. We measured CO₂ efflux from the floors and walls of shrimp ponds. Rates of CO₂ efflux within shrimp ponds were 4.37 kg CO₂ m⁻² y⁻¹ from the walls and 1.60 kg CO₂ m⁻² y⁻¹ from the floors. Combining our findings with published data of aquaculture land use in Indonesia, we estimated that shrimp ponds in this region result in CO₂ emissions to the atmosphere between 5.76 and 13.95 Tg y⁻¹. The results indicate that conversion of mangrove forests to aquaculture ponds contributes to greenhouse gas emissions that are comparable to peat forest conversion to other land uses in Indonesia. Higher magnitudes of CO₂ emission may be released to atmosphere where ponds are constructed in newly cleared mangrove forests. This study indicates the need for incentives that can meet the target of aquaculture industry without expanding the converted mangrove areas, which will lead to increased CO₂ released to atmosphere.

ENVIRONMENTAL CHAMBER STUDIES OF MERCURY REACTIONS IN THE ATMOSPHERE

EPA Science Inventory

Mercury is released into the environment through both natural and anthropogenic pathways. The cycling and fate of mercury in atmospheric, soil, and water ecosystems is impacted by various factors, including chemical transformation and transport. An understanding of these proces...

Defense Coastal/Estuarine Research Program (DCERP) Strategic Plan

DTIC Science & Technology

2007-09-01

atmospheric deposition. The source apportionment of nutrients from atmospheric deposition (especially nitrogen) to estuarine waters derived from direct...migrating wildlife, and nutrient release from soil weathering, atmospheric deposition represents the only source of new nutrients into the... apportionment to properly assess the contributions of off-site and on-site emission sources to regional levels of PM2.5. In preparing this DCERP Strategic

Environmental change and the conversion of permanently frozen ground to wetlands

NASA Astrophysics Data System (ADS)

Neumann, R. B.; Moorberg, C.; Turner, J.; Wong, A.; Waldrop, M. P.; Euskirchen, E. S.; Edgar, C.; Turetsky, M. R.

2017-12-01

Much of the land around the arctic is permanently frozen, even in the summer. However, because the world is getting warmer, this frozen ground, known as permafrost, is thawing. When permafrost thaws, the ground collapses and sinks, and often a wetland forms within the collapsed area. This conversion of a permanently frozen landscape to a wetland changes the exchange of greenhouse gases between the land and atmosphere, which can, in turn, impact global temperatures and environmental conditions. Wetlands pull carbon dioxide out of the atmosphere because they support the growth of many plants. This uptake of atmospheric carbon dioxide by wetlands helps reduce global warming. However, wetlands also release methane into the atmosphere, which is a potent greenhouse gas — more potent than carbon dioxide. The net effect on global temperatures and environmental conditions depends on the balance between wetland uptake of atmospheric carbon dioxide and release of methane. We are measuring the exchange of these two greenhouse gases between the land and atmosphere in a wetland that formed after permafrost thawed so we can know how global temperatures and environmental conditions will change as northern landscapes continue to thaw.

RIM-BPs Mediate Tight Coupling of Action Potentials to Ca(2+)-Triggered Neurotransmitter Release.

PubMed

Acuna, Claudio; Liu, Xinran; Gonzalez, Aneysis; Südhof, Thomas C

2015-09-23

Ultrafast neurotransmitter release requires tight colocalization of voltage-gated Ca(2+) channels with primed, release-ready synaptic vesicles at the presynaptic active zone. RIM-binding proteins (RIM-BPs) are multidomain active zone proteins that bind to RIMs and to Ca(2+) channels. In Drosophila, deletion of RIM-BPs dramatically reduces neurotransmitter release, but little is known about RIM-BP function in mammalian synapses. Here, we generated double conditional knockout mice for RIM-BP1 and RIM-BP2, and analyzed RIM-BP-deficient synapses in cultured hippocampal neurons and the calyx of Held. Surprisingly, we find that in murine synapses, RIM-BPs are not essential for neurotransmitter release as such, but are selectively required for high-fidelity coupling of action potential-induced Ca(2+) influx to Ca(2+)-stimulated synaptic vesicle exocytosis. Deletion of RIM-BPs decelerated action-potential-triggered neurotransmitter release and rendered it unreliable, thereby impairing the fidelity of synaptic transmission. Thus, RIM-BPs ensure optimal organization of the machinery for fast release in mammalian synapses without being a central component of the machinery itself. Copyright © 2015 Elsevier Inc. All rights reserved.

Modelling the effect of soil moisture and organic matter degradation on biogenic NO emissions from soils in Sahel rangeland (Mali)

NASA Astrophysics Data System (ADS)

Delon, C.; Mougin, E.; Serça, D.; Grippa, M.; Hiernaux, P.; Diawara, M.; Galy-Lacaux, C.; Kergoat, L.

2015-06-01

This work is an attempt to provide seasonal variation of biogenic NO emission fluxes in a Sahelian rangeland in Mali (Agoufou, 15.34° N, 1.48° W) for years 2004, 2005, 2006, 2007 and 2008. Indeed, NO is one of the most important precursors for tropospheric ozone, and previous studies have shown that arid areas potentially display significant NO emissions (due to both biotic and abiotic processes). Previous campaigns in the Sahel suggest that the contribution of this region in emitting NO is no longer considered as negligible. However, very few data are available in this region, therefore this study focuses on model development. The link between NO production in the soil and NO release to the atmosphere is investigated in this modelling study, by taking into account vegetation litter production and degradation, microbial processes in the soil, emission fluxes, and environmental variables influencing these processes, using a coupled vegetation-litter decomposition-emission model. This model includes the Sahelian Transpiration Evaporation and Productivity (STEP) model for the simulation of herbaceous, tree leaf and faecal masses, the GENDEC model (GENeral DEComposition) for the simulation of the buried litter decomposition and microbial dynamics, and the NO emission model (NOFlux) for the simulation of the NO release to the atmosphere. Physical parameters (soil moisture and temperature, wind speed, sand percentage) which affect substrate diffusion and oxygen supply in the soil and influence the microbial activity, and biogeochemical parameters (pH and fertilization rate related to N content) are necessary to simulate the NO flux. The reliability of the simulated parameters is checked, in order to assess the robustness of the simulated NO flux. Simulated yearly average of NO flux ranges from 2.09 to 3.04 ng(N) m-2 s-1 (0.66 to 0.96 kg(N) ha-1 yr-1), and wet season average ranges from 3.36 to 5.48 ng(N) m-2 s-1 (1.06 to 1.73 kg(N) ha-1 yr-1). These results are of the same order as previous measurements made in several sites where the vegetation and the soil are comparable to the ones in Agoufou. This coupled vegetation-litter decomposition-emission model could be generalized at the scale of the Sahel region, and provide information where few data are available.

Incorporating JULES into NASA's Land Information System (LIS) and Investigations of Land-Atmosphere Coupling

NASA Technical Reports Server (NTRS)

Santanello, Joseph

2011-01-01

NASA's Land Information System (LIS; lis.gsfc.nasa.gov) is a flexible land surface modeling and data assimilation framework developed over the past decade with the goal of integrating satellite- and ground-based observational data products and advanced land surface modeling techniques to produce optimal fields of land surface states and fluxes. LIS features a high performance and flexible design, and operates on an ensemble of land surface models for extension over user-specified regional or global domains. The extensible interfaces of LIS allow the incorporation of new domains, land surface models (LSMs), land surface parameters, meteorological inputs, data assimilation and optimization algorithms. In addition, LIS has also been demonstrated for parameter estimation and uncertainty estimation, and has been coupled to the Weather Research and Forecasting (WRF) mesoscale model. A visiting fellowship is currently underway to implement JULES into LIS and to undertake some fundamental science on the feedbacks between the land surface and the atmosphere. An overview of the LIS system, features, and sample results will be presented in an effort to engage the community in the potential advantages of LIS-JULES for a range of applications. Ongoing efforts to develop a framework for diagnosing land-atmosphere coupling will also be presented using the suite of LSM and PBL schemes available in LIS and WRF along with observations from the U. S .. Southern Great Plains. This methodology provides a potential pathway to study factors controlling local land-atmosphere coupling (LoCo) using the LIS-WRF system, which will serve as a testbed for future experiments to evaluate coupling diagnostics within the community.

Corrective Action Investigation Plan for Corrective Action Unit 104: Area 7 Yucca Flat Atmospheric Test Sites, Nevada National Security Site, Nevada, Revision 0

DOE Office of Scientific and Technical Information (OSTI.GOV)

Patrick Matthews

2011-08-01

CAU 104 comprises the 15 CASs listed below: (1) 07-23-03, Atmospheric Test Site T-7C; (2) 07-23-04, Atmospheric Test Site T7-1; (3) 07-23-05, Atmospheric Test Site; (4) 07-23-06, Atmospheric Test Site T7-5a; (5) 07-23-07, Atmospheric Test Site - Dog (T-S); (6) 07-23-08, Atmospheric Test Site - Baker (T-S); (7) 07-23-09, Atmospheric Test Site - Charlie (T-S); (8) 07-23-10, Atmospheric Test Site - Dixie; (9) 07-23-11, Atmospheric Test Site - Dixie; (10) 07-23-12, Atmospheric Test Site - Charlie (Bus); (11) 07-23-13, Atmospheric Test Site - Baker (Buster); (12) 07-23-14, Atmospheric Test Site - Ruth; (13) 07-23-15, Atmospheric Test Site T7-4; (14) 07-23-16,more » Atmospheric Test Site B7-b; (15) 07-23-17, Atmospheric Test Site - Climax These sites are being investigated because existing information on the nature and extent of potential contamination is insufficient to evaluate and recommend corrective action alternatives (CAAs). Additional information will be obtained by conducting a corrective action investigation before evaluating CAAs and selecting the appropriate corrective action for each CAS. The results of the field investigation will support a defensible evaluation of viable CAAs that will be presented in the Corrective Action Decision Document. The sites will be investigated based on the data quality objectives (DQOs) developed on April 28, 2011, by representatives of the Nevada Division of Environmental Protection and the U.S. Department of Energy (DOE), National Nuclear Security Administration Nevada Site Office. The DQO process was used to identify and define the type, amount, and quality of data needed to develop and evaluate appropriate corrective actions for CAU 104. The releases at CAU 104 consist of surface-deposited radionuclides from 30 atmospheric nuclear tests. The presence and nature of contamination at CAU 104 will be evaluated based on information collected from a field investigation. Radiological contamination will be evaluated based on a comparison of the total effective dose (TED) to the dose-based final action level (FAL). The presence of TED exceeding the FAL is considered a radiological contaminant of concern (COC). Anything identified as a COC will require corrective action. The TED will be calculated as the total of separate estimates of internal and external dose. Results from the analysis of soil samples will be used to calculate internal radiological dose. Thermoluminescent dosimeters will be used to measure external radiological dose. Based on process knowledge of the releases associated with the nuclear tests and radiological survey information about the location and shape of the resulting contamination plume, it was determined that the releases from the nuclear tests are co-located and will be investigated concurrently. A field investigation will be performed to define areas where TED exceeds the FAL and to determine whether other COCs are present at the site. The investigation will also collect information to determine the presence and nature of contamination associated with migration and excavation, as well as any potential releases discovered during the investigation. Appendix A provides a detailed discussion of the DQO methodology and the DQOs specific to each CAS.« less