Dynamics of near-surface electric discharges and mechanisms of their interaction with the airflow

NASA Astrophysics Data System (ADS)

Leonov, Sergey B.; Adamovich, Igor V.; Soloviev, Victor R.

2016-12-01

The main focus of the review is on dynamics and kinetics of near-surface discharge plasmas, such as surface dielectric barrier discharges sustained by AC and repetitively pulsed waveforms, pulsed DC discharges, and quasi-DC discharges, generated in quiescent air and in the airflow. A number of technical issues related to plasma flow control applications are discussed in detail, including discharge development via surface ionization waves, charge transport and accumulation on dielectric surface, discharge contraction, different types of flow perturbations generated by surface discharges, and effect of high-speed flow on discharge dynamics. In the first part of the manuscript, plasma morphology and results of electrical and optical emission spectroscopy measurements are discussed. Particular attention is paid to dynamics of surface charge accumulation and dissipation, both in diffuse discharges and during development of ionization instabilities resulting in discharge contraction. Contraction leads to significant increase of both the surface area of charge accumulation and the energy coupled to the plasma. The use of alternating polarity pulse waveforms accelerates contraction of surface dielectric barrier discharges and formation of filamentary plasmas. The second part discusses the interaction of discharge plasmas with quiescent air and the external airflow. Four major types of flow perturbations have been identified: (1) low-speed near-surface jets generated by electrohydrodynamic interaction (ion wind); (2) spanwise and streamwise vortices formed by both electrohydrodynamic and thermal effects; (3) weak shock waves produced by rapid heating in pulsed discharges on sub-microsecond time scale; and (4) near-surface localized stochastic perturbations, on sub-millisecond time, detected only recently. The mechanism of plasma-flow interaction remains not fully understood, especially in filamentary surface dielectric barrier discharges. Localized quasi-DC surface discharges sustained in a high-speed flow are discussed in the third part of the review. Although dynamics of this type of the discharge is highly transient, due to its strong interaction with the flow, the resultant flow structure is stationary, including the oblique shock and the flow separation region downstream of the discharge. The oblique shock is attached to a time-averaged, wedge-shaped, near-wall plasma layer, with the shock angle controlled by the discharge power, which makes possible changing the flow structure and parameters in a controlled way. Finally, unresolved and open-ended issues are discussed in the summary.

Hollow-Cathode Source Generates Plasma

NASA Technical Reports Server (NTRS)

Deininger, W. D.; Aston, G.; Pless, L. C.

1989-01-01

Device generates argon, krypton, or xenon plasma via thermionic emission and electrical discharge within hollow cathode and ejects plasma into surrounding vacuum. Goes from cold start up to full operation in less than 5 s after initial application of power. Exposed to moist air between operations without significant degradation of starting and running characteristics. Plasma generated by electrical discharge in cathode barrel sustained and aided by thermionic emission from emitter tube. Emitter tube does not depend on rare-earth oxides, making it vulnerable to contamination by exposure to atmosphere. Device modified for use as source of plasma in laboratory experiments or industrial processes.

Kinetics and Chemistry of Ionization Wave Discharges Propagating Over Dielectric Surfaces

NASA Astrophysics Data System (ADS)

Petrishchev, Vitaly

Experimental studies of near-surface ionization wave electric discharges generated by high peak voltage (20-30 kV), nanosecond duration pulses (full width at half-maximum 50-100 ns) of positive and negative polarity and propagating over dielectric surfaces have been performed. A novel way to sustain diffuse, reproducible, ns pulse surface plasmas at a liquid-vapor interface is demonstrated at buffer gas pressures ranging from 10 to 200 Torr. Generation of surface ionization waves well reproduced shot-to-shot and sustaining diffuse near-surface plasmas is one of the principal advantages of the use of ns pulse discharge waveforms. This makes possible characterization of these plasmas in repetitively pulsed experiments. Numerous applications of these plasmas include low-temperature plasma assisted combustion, plasma fuel reforming, plasma flow control, plasma materials processing, agriculture, biology, and medicine. The objectives of the present work are (i) to demonstrate that surface ionization wave discharge plasmas sustained at a liquid-vapor interface can be used as an experimental platform for studies of near-surface plasma chemical reaction kinetics, at the conditions when the interface acts as a high-yield source of radical species, and (ii) to obtain quantitative insight into dynamics, kinetics and chemistry of surface ionization wave discharges and provide experimental data for validation of kinetic models, to assess their predictive capability. Generation of the initial radical pool may trigger a number of plasma chemical processes leading to formation of a variety of stable product species, depending on the initial composition of the liquid and the buffer gas flow. One of the products formed and detected during surface plasma / liquid water interaction is hydroxyl radical, which is closely relevant to applications of plasmas for biology and medicine. The present work includes detailed studies of surface ionization wave discharges sustained in different buffer gases over solid and liquid dielectric surfaces, such as quartz, distilled water, saline solution, and alcohols, over a wide range of pressures. Specific experiments include: measurements of ionization wave speed; plasma emission imaging using a ns gate camera; detection of surface discharge plasma chemistry products using Fourier transform infrared absorption spectroscopy; surface charge dynamics on short (ns) and long (hundreds of mus) time scales; time-resolved electron density and electron temperature measurements in a ns pulse surface discharge in helium by Thomson scattering; spatially-resolved absolute OH and H atom concentration measurements in ns pulse discharges over distilled water by single-photon and two-photon Laser Induced Fluorescence; and schlieren imaging of perturbations generated by a ns pulse dielectric barrier discharge in a surface plasma actuator in quiescent atmospheric pressure air.

A Multiple Z-Pinch Configuration for the Generation of High-Density, Magnetized Plasmas

NASA Astrophysics Data System (ADS)

Tarditi, Alfonso G.

2015-11-01

The z-pinch is arguably the most straightforward and economical approach for the generation and confinement of hot plasmas, with a long history of theoretical investigations and experimental developments. While most of the past studies were focused on countering the natural tendency of z-pinches to develop instabilities, this study attempts to take advantage of those unstable regimes to form a quasi-stable plasma, with higher density and temperature, possibly of interest for a fusion reactor concept. For this purpose, a configuration with four z-pinch discharges, with axis parallel to each other and symmetrically positioned, is considered. Electrodes for the generation of the discharges and magnetic coils are arranged to favor the formation of concave discharge patterns. The mutual attraction from the co-streaming discharge currents enhances this pattern, leading to bent plasma streams, all nearing towards the axis. This configuration is intended to excite and sustain a ``kink'' unstable mode for each z-pinch, eventually producing either plasmoid structures, detached from each discharge, or sustained kink patterns: both these cases appear to lead to plasmas merging in the central region. The feasibility of this approach in creating a higher density, hotter, meta-stable plasma regime is investigated computationally, addressing both the kink excitation phase and the dynamics of the converging plasma columns.

A linear-field plasma jet for generating a brush-shaped laminar plume at atmospheric pressure

DOE Office of Scientific and Technical Information (OSTI.GOV)

Li, Xuechen; Jia, Pengying, E-mail: plasmalab@126.com; Key Laboratory of Photo-Electronics Information Materials of Hebei Province, Baoding 071002

2016-06-15

A linear-field plasma jet composed of line-to-plate electrodes is used to generate a large-scale brush-shaped plasma plume with flowing argon used as working gas. Through electrical measurement and fast photography, it is found that the plasma plume bridges the two electrodes for the discharge in the positive voltage half-cycle, which behaves like fast moving plasma bullets directed from the anode to the cathode. Compared with the positive discharge, the negative discharge only develops inside the nozzle and propagates much slower. Results also indicate that the gas temperature of the plume is close to room temperature, which is promising for biomedicalmore » application.« less

Plasma treatment of polyethylene tubes in continuous regime using surface dielectric barrier discharge with water electrodes

NASA Astrophysics Data System (ADS)

Galmiz, Oleksandr; Zemánek, Miroslav; Pavliňák, David; Černák, Mirko

2018-05-01

Combining the surface dielectric barrier discharges generated in contact with water based electrolytes, as the discharge electrodes, we have designed a new type of surface electric discharge, generating thin layers of plasma which propagate along the treated polymer surfaces. The technique was aimed to achieve uniform atmospheric pressure plasma treatment of polymeric tubes and other hollow bodies. The results presented in this work show the possibility of such system to treat outer surface of polymer materials in a continuous mode. The technical details of experimental setup are discussed as well as results of treatment of polyethylene tubes are shown.

Production of atmospheric pressure diffuse nanosecond pulsed dielectric barrier discharge using the array needles-plate electrode in air

NASA Astrophysics Data System (ADS)

Yang, De-zheng; Wang, Wen-chun; Jia, Li; Nie, Dong-xia; Shi, Heng-chao

2011-04-01

In this paper, a bidirectional high pulse voltage with 20 ns rising time is employed to generate an atmospheric pressure diffuse dielectric barrier discharge using the array needles-plate electrode configuration. Both double needle and multiple needle electrode configurations nanosecond pulsed dielectric barrier discharges are investigated. It is found that a diffuse discharge plasma with low gas temperature can be obtained, and the plasma volume increases with the increase of the pulse peak voltage, but remains almost constant with the increase of the pulse repetition rate. In addition to showing the potential application on a topographically nonuniform surface treatment of the discharge, the multiple needle-plate electrode configuration with different needle-plate electrode gaps are also employed to generate diffuse discharge plasma.

Plasma in a Pulsed Discharge Environment

NASA Technical Reports Server (NTRS)

Remy, J.; Bienier, L.; Salama, F.

2005-01-01

The plasma generated in a pulsed slit discharge nozzle is used to form molecular ions in an astrophysically relevant environment. The plasma has been characterized as a glow discharge in the abnormal regime. Laboratory studies help understand the formation processes of polycyclic aromatic hydrocarbon (PAH) ions that are thought to be the source of the ubiquitous unidentified infrared bands.

Plasma discharge self-cleaning filtration system

DOEpatents

Cho, Young I.; Fridman, Alexander; Gutsol, Alexander F.; Yang, Yong

2014-07-22

The present invention is directed to a novel method for cleaning a filter surface using a plasma discharge self-cleaning filtration system. The method involves utilizing plasma discharges to induce short electric pulses of nanoseconds duration at high voltages. These electrical pulses generate strong Shockwaves that disintegrate and dislodge particulate matter located on the surface of the filter.

Method for generating a highly reactive plasma for exhaust gas aftertreatment and enhanced catalyst reactivity

DOEpatents

Whealton, John H.; Hanson, Gregory R.; Storey, John M.; Raridon, Richard J.; Armfield, Jeffrey S.; Bigelow, Timothy S.; Graves, Ronald L.

2001-01-01

A method for non-thermal plasma aftertreatment of exhaust gases the method comprising the steps of providing short risetime (about 40 ps), high frequency (about 5G hz), high power bursts of low-duty factor microwaves sufficient to generate a dielectric barrier discharge and passing a gas to treated through the discharge so as to cause dissociative reduction of the exhaust gases. The invention also includes a reactor for generating the non-thermal plasma.

FAST TRACK COMMUNICATION: Effects of Penning ionization on the discharge patterns of atmospheric pressure plasma jets

NASA Astrophysics Data System (ADS)

Li, Qing; Zhu, Wen-Chao; Zhu, Xi-Ming; Pu, Yi-Kang

2010-09-01

Atmospheric pressure plasma jets, generated in a coaxial dielectric barrier discharge configuration, have been investigated with different flowing gases. Discharge patterns in different tube regions were compared in the flowing gases of helium, neon and krypton. To explain the difference of these discharge patterns, a theoretical analysis is presented to reveal the possible basic processes. A comparison of experimental and theoretical results identifies that Penning ionization is mainly responsible for the discharge patterns of helium and neon plasma jets.

Review of electric discharge microplasmas generated in highly fluctuating fluids: Characteristics and application to nanomaterials synthesis

DOE Office of Scientific and Technical Information (OSTI.GOV)

Stauss, Sven, E-mail: sven.stauss@plasma.k.u-tokyo.ac.jp; Terashima, Kazuo, E-mail: kazuo@plasma.k.u-tokyo.ac.jp; Muneoka, Hitoshi

2015-05-15

Plasma-based fabrication of novel nanomaterials and nanostructures is indispensible for the development of next-generation electronic devices and for green energy applications. In particular, controlling the interactions between plasmas and materials interfaces, and the plasma fluctuations, is crucial for further development of plasma-based processes and bottom-up growth of nanomaterials. Electric discharge microplasmas generated in supercritical fluids represent a special class of high-pressure plasmas, where fluctuations on the molecular scale influence the discharge properties and the possible bottom-up growth of nanomaterials. This review discusses an anomaly observed for direct current microplasmas generated near the critical point, a local decrease in the breakdownmore » voltage. This anomalous behavior is suggested to be caused by the concomitant decrease of the ionization potential due to the formation of clusters near the critical point, and the formation of extended electron mean free paths caused by the high-density fluctuation near the critical point. It is also shown that in the case of dielectric barrier microdischarges generated close to the critical point, the high-density fluctuation of the supercritical fluid persists. The final part of the review discusses the application of discharges generated in supercritical fluids to synthesis of nanomaterials, in particular, molecular diamond—so-called diamondoids—by microplasmas generated inside conventional batch-type and continuous flow microreactors.« less

Discharge Characteristics of DC Arc Water Plasma for Environmental Applications

NASA Astrophysics Data System (ADS)

Li, Tianming; Sooseok, Choi; Takayuki, Watanabe

2012-12-01

A water plasma was generated by DC arc discharge with a hafnium embedded rod-type cathode and a nozzle-type anode. The discharge characteristics were examined by changing the operation parameter of the arc current. The dynamic behavior of the arc discharge led to significant fluctuations in the arc voltage and its frequency. Analyses of the high speed image and the arc voltage waveform showed that the arc discharge was in the restrike mode and its frequency varied within several tens of kilohertz according to the operating conditions. The larger thermal plasma volume was generated by the higher flow from the forming steam with a higher restrike frequency in the higher arc current conditions. In addition, the characteristics of the water plasma jet were investigated by means of optical emission spectroscopy to identify the abundant radicals required in an efficient waste treatment process.

Process Performances of 2 ns Pulsed Discharge Plasma

NASA Astrophysics Data System (ADS)

Matsumoto, Takao; Wang, Douyan; Namihira, Takao; Akiyama, Hidenori

2011-08-01

Pulsed discharge plasmas have been used to treat exhaust gases. Since pulse duration and the rise time of applied voltage to the discharge electrode has a strong influence on the energy efficiency of pollutant removal, the development of a short-pulse generator is of paramount importance for practical applications. In this work, it is demonstrated that the non thermal plasma produced by the 2 ns pulsed discharge has a higher energy efficiency than the 5 ns pulsed discharge plasma for NO removal and ozone generation. Typically, the NO removal efficiency was 1.0 mol kW-1 h-1 for 70% NO removal (initial NO concentration = 200 ppm, gas flow = 10 L/min). Meanwhile, the ozone yield was 500 g kW-1 h-1 for 20 g/m3 ozone concentration in the case of oxygen feeding. These energy efficiencies are the highest in the literature.

Characteristics of electromagnetic interference generated by arc discharges. [in spacecraft

NASA Technical Reports Server (NTRS)

Leung, Philip

1986-01-01

Electromagnetic interference (EMI) signatures resulting from arc discharges are characterized, and the effects of electrostatic discharges (ESDs) on the design of spacecraft systems are investigated. EMI characterization experiments were performed on Mylar, Teflon, Kapton, fused silica, and fiberglass in a vacuum chamber with acrylic walls; the experimental design and procedures are described. Discharge current pulses and RF spectra generated by the sample materials are examined. The relation between the magnitude of EMI generated during an ESD event and the material, environment, and geometry is studied. The solar-array/plasma interaction is analyzed; particular attention is given to the rate of discharge as a function of plasma density. The physical mechanisms of ESD-generated EMI are discussed. The data reveal that ESD parameters are dependent on the test environment.

Introduction of Nano-seconds Pulsed Discharge Plasma and its Applications

NASA Astrophysics Data System (ADS)

Namihira, Takao; Wang, Douyan; Matsumoto, Takao; Okada, Sho; Akiyama, Hidenori

During the decades, the developments of high power semiconductor switch, magnetic core and etc have allowed us to manufacture the pulsed power source having higher energy transfer efficiency. As the results, the pulsed discharge has been recognized as one of the promised non-thermal plasma to practical use. In this paper, a generation process, electron energy, impedance and a temperature of the pulsed discharge plasma would be explained. In addition, a nano-seconds pulsed discharge plasma would be introduced as the non-thermal plasma processing giving us the highest energy efficiency and be demonstrated it.

Comparison of plasma generated nitrogen fertilizer to conventional fertilizers ammonium nitrate and sodium nitrate for pre-emergent and seedling growth

NASA Astrophysics Data System (ADS)

Andhavarapu, A.; King, W.; Lindsay, A.; Byrns, B.; Knappe, D.; Fonteno, W.; Shannon, S.

2014-10-01

Plasma source generated nitrogen fertilizer is compared to conventional nitrogen fertilizers in water for plant growth. Root, shoot sizes, and weights are used to examine differences between plant treatment groups. With a simple coaxial structure creating a large-volume atmospheric glow discharge, a 162 MHz generator drives the air plasma. The VHF plasma source emits a steady state glow; the high drive frequency is believed to inhibit the glow-to-arc transition for non-thermal discharge generation. To create the plasma activated water (PAW) solutions used for plant treatment, the discharge is held over distilled water until a 100 ppm nitrate aqueous concentration is achieved. The discharge is used to incorporate nitrogen species into aqueous solution, which is used to fertilize radishes, marigolds, and tomatoes. In a four week experiment, these plants are watered with four different solutions: tap water, dissolved ammonium nitrate DI water, dissolved sodium nitrate DI water, and PAW. Ammonium nitrate solution has the same amount of total nitrogen as PAW; sodium nitrate solution has the same amount of nitrate as PAW. T-tests are used to determine statistical significance in plant group growth differences. PAW fertilization chemical mechanisms are presented.

Boron hydride polymer coated substrates

DOEpatents

Pearson, R.K.; Bystroff, R.I.; Miller, D.E.

1986-08-27

A method is disclosed for coating a substrate with a uniformly smooth layer of a boron hydride polymer. The method comprises providing a reaction chamber which contains the substrate and the boron hydride plasma. A boron hydride feed stock is introduced into the chamber simultaneously with the generation of a plasma discharge within the chamber. A boron hydride plasma of ions, electrons and free radicals which is generated by the plasma discharge interacts to form a uniformly smooth boron hydride polymer which is deposited on the substrate.

Boron hydride polymer coated substrates

DOEpatents

Pearson, Richard K.; Bystroff, Roman I.; Miller, Dale E.

1987-01-01

A method is disclosed for coating a substrate with a uniformly smooth layer of a boron hydride polymer. The method comprises providing a reaction chamber which contains the substrate and the boron hydride plasma. A boron hydride feed stock is introduced into the chamber simultaneously with the generation of a plasma discharge within the chamber. A boron hydride plasma of ions, electrons and free radicals which is generated by the plasma discharge interacts to form a uniformly smooth boron hydride polymer which is deposited on the substrate.

Megawatt low-temperature DC plasma generator with divergent channels of gas-discharge tract

NASA Astrophysics Data System (ADS)

Gadzhiev, M. Kh.; Isakaev, E. Kh.; Tyuftyaev, A. S.; Yusupov, D. I.; Sargsyan, M. A.

2017-04-01

We have developed and studied a new effective megawatt double-unit generator of low-temperature argon plasma, which belongs to the class of dc plasmatrons and comprises the cathode and anode units with divergent gas-discharge channels. The generator has an efficiency of about 80-85% and ensures a long working life at operating currents up to 4000 A.

Review of the methods to form hydrogen peroxide in electrical discharge plasma with liquid water

NASA Astrophysics Data System (ADS)

Locke, Bruce R.; Shih, Kai-Yuan

2011-06-01

This paper presents a review of the literature dealing with the formation of hydrogen peroxide from plasma processes. Energy yields for hydrogen peroxide generation by plasma from water span approximately three orders of magnitude from 4 × 10-2 to 80 g kWh-1. A wide range of plasma processes from rf to pulsed, ac, and dc discharges directly in the liquid phase have similar energy yields and may thus be limited by radical quenching processes at the plasma-liquid interface. Reactor modification using discharges in bubbles and discharges over the liquid phase can provide modest improvements in energy yield over direct discharge in the liquid, but the interpretation is complicated by additional chemical reactions of gas phase components such as ozone and nitrogen oxides. The highest efficiency plasma process utilizes liquid water droplets that may enhance efficiency by sequestering hydrogen peroxide in the liquid and by suppressing decomposition reactions by radicals from the gas and at the interface. Kinetic simulations of water vapor reported in the literature suggest that plasma generation of hydrogen peroxide should approach 45% of the thermodynamics limit, and this fact coupled with experimental studies demonstrating improvements with the presence of the condensed liquid phase suggest that further improvements in energy yield may be possible. Plasma generation of hydrogen peroxide directly from water compares favorably with a number of other methods including electron beam, ultrasound, electrochemical and photochemical methods, and other chemical processes.

A compact nanosecond pulse generator for DBD tube characterization.

PubMed

Rai, S K; Dhakar, A K; Pal, U N

2018-03-01

High voltage pulses of very short duration and fast rise time are required for generating uniform and diffuse plasma under various operating conditions. Dielectric Barrier Discharge (DBD) has been generated by high voltage pulses of short duration and fast rise time to produce diffuse plasma in the discharge gap. The high voltage pulse power generators have been chosen according to the requirement for the DBD applications. In this paper, a compact solid-state unipolar pulse generator has been constructed for characterization of DBD plasma. This pulsar is designed to provide repetitive pulses of 315 ns pulse width, pulse amplitude up to 5 kV, and frequency variation up to 10 kHz. The amplitude of the output pulse depends on the dc input voltage. The output frequency has been varied by changing the trigger pulse frequency. The pulsar is capable of generating pulses of positive or negative polarity by changing the polarity of pulse transformer's secondary. Uniform and stable homogeneous dielectric barrier discharge plasma has been produced successfully in a xenon DBD tube at 400-mbar pressure using the developed high voltage pulse generator.

A compact nanosecond pulse generator for DBD tube characterization

NASA Astrophysics Data System (ADS)

Rai, S. K.; Dhakar, A. K.; Pal, U. N.

2018-03-01

High voltage pulses of very short duration and fast rise time are required for generating uniform and diffuse plasma under various operating conditions. Dielectric Barrier Discharge (DBD) has been generated by high voltage pulses of short duration and fast rise time to produce diffuse plasma in the discharge gap. The high voltage pulse power generators have been chosen according to the requirement for the DBD applications. In this paper, a compact solid-state unipolar pulse generator has been constructed for characterization of DBD plasma. This pulsar is designed to provide repetitive pulses of 315 ns pulse width, pulse amplitude up to 5 kV, and frequency variation up to 10 kHz. The amplitude of the output pulse depends on the dc input voltage. The output frequency has been varied by changing the trigger pulse frequency. The pulsar is capable of generating pulses of positive or negative polarity by changing the polarity of pulse transformer's secondary. Uniform and stable homogeneous dielectric barrier discharge plasma has been produced successfully in a xenon DBD tube at 400-mbar pressure using the developed high voltage pulse generator.

Sustained diffusive alternating current gliding arc discharge in atmospheric pressure air

NASA Astrophysics Data System (ADS)

Zhu, Jiajian; Gao, Jinlong; Li, Zhongshan; Ehn, Andreas; Aldén, Marcus; Larsson, Anders; Kusano, Yukihiro

2014-12-01

Rapid transition from glow discharge to thermal arc has been a common problem in generating stable high-power non-thermal plasmas especially at ambient conditions. A sustained diffusive gliding arc discharge was generated in a large volume in atmospheric pressure air, driven by an alternating current (AC) power source. The plasma column extended beyond the water-cooled stainless steel electrodes and was stabilized by matching the flow speed of the turbulent air jet with the rated output power. Comprehensive investigations were performed using high-speed movies measured over the plasma column, synchronized with simultaneously recorded current and voltage waveforms. Dynamic details of the novel non-equilibrium discharge are revealed, which is characterized by a sinusoidal current waveform with amplitude stabilized at around 200 mA intermediate between thermal arc and glow discharge, shedding light to the governing mechanism of the sustained spark-suppressed AC gliding arc discharge.

Control of plasma-liquid interaction of atmospheric DC glow discharge using liquid electrode

NASA Astrophysics Data System (ADS)

Shirai, Naoki; Aoki, Ryuta; Nito, Aihito; Aoki, Takuya; Uchida, Satoshi; Tochikubo, Fumiyoshi

2014-10-01

Atmospheric plasma in contact with liquid have a variety of interesting phenomena and applications. Previously, we investigated the fundamental characteristics of an atmospheric dc glow discharge using a liquid electrode with a miniature helium flow. We tried to control the plasma-liquid interaction by changing the plasma parameter such as gas species, liquid, and applied voltage. Sheath flow system enables another gas (N2, O2, Ar) flow to around the helium core flow. It can control the gas species around the discharge. When liquid (NaCl aq.) cathode DC discharge is generated, Na emission (588 nm) can be observed from liquid surface with increasing discharge current. Na emission strongly depends on the discharge current and liquid temperature. However, when Ar sheath flow is used, the intensity of Na becomes weak. When liquid anode DC discharge is generated, self-organized luminous pattern formation can be observed at the liquid surface. The pattern depends on existence of oxygen gas in gap. By changing the oxygen gas ratio in the gap, variety of pattern formation can be observed. The discharge in contact with liquid also can be used for synthesis of metal nanoparticles at plasma-liquid interface. Size and shape of nanoparticles depend on discharge gases. This work was supported financially in part by a Grant-in-Aid for Scientific Research on Innovative Areas (No 21110007) from MEXT, Japan.

Aqueous Plasma Pharmacy: Preparation Methods, Chemistry, and Therapeutic Applications

PubMed Central

Joslin, Jessica M.; McCall, James R.; Bzdek, Justin P.; Johnson, Derek C.; Hybertson, Brooks M.

2017-01-01

Plasma pharmacy is a subset of the broader field of plasma medicine. Although not strictly defined, the term aqueous plasma pharmacy (APP) is used to refer to the generation and distribution of reactive plasma-generated species in an aqueous solution followed by subsequent administration for therapeutic benefits. APP attempts to harness the therapeutic effects of plasma-generated oxidant species within aqueous solution in various applications, such as disinfectant solutions, cell proliferation related to wound healing, and cancer treatment. The subsequent use of plasma-generated solutions in the APP approach facilitates the delivery of reactive plasma species to internal locations within the body. Although significant efforts in the field of plasma medicine have concentrated on employing direct plasma plume exposure to cells or tissues, here we focus specifically on plasma discharge in aqueous solution to render the solution biologically active for subsequent application. Methods of plasma discharge in solution are reviewed, along with aqueous plasma chemistry and the applications for APP. The future of the field also is discussed regarding necessary research efforts that will enable commercialization for clinical deployment. PMID:28428835

Needle-array to Plate DBD Plasma Using Sine AC and Nanosecond Pulse Excitations for Purpose of Improving Indoor Air Quality

PubMed Central

Zhang, Li; Yang, Dezheng; Wang, Wenchun; Wang, Sen; Yuan, Hao; Zhao, Zilu; Sang, Chaofeng; Jia, Li

2016-01-01

In this study, needle-array to plate electrode configuration was employed to generate an atmospheric air diffuse discharge using both nanosecond pulse and sine AC voltage as excitation voltage for the purpose of improving indoor air quality. Different types of voltage sources and electrode configurations are employed to optimize electrical field distribution and improve discharge stability. Discharge images, electrical characteristics, optical emission spectra, and plasma gas temperatures in both sine AC discharge and nanosecond pulse discharge were compared and the discharge stability during long operating time were discussed. Compared with the discharge excited by sine AC voltage, the nanosecond pulsed discharge is more homogenous and stable, besides, the plasma gas temperature of nanosecond pulse discharge is much lower. Using packed-bed structure, where γ- Al2O3 pellets are filled in the electrode gap, has obvious efficacy in the production of homogenous discharge. Furthermore, both sine AC discharge and nanosecond pulse discharge were used for removing formaldehyde from flowing air. It shows that nanosecond pulse discharge has a significant advantage in energy cost. And the main physiochemical processes for the generation of active species and the degradation of formaldehyde were discussed. PMID:27125663

Atmospheric-pressure electric discharge as an instrument of chemical activation of water solutions

NASA Astrophysics Data System (ADS)

Rybkin, V. V.; Shutov, D. A.

2017-11-01

Results of experimental studies and numerical simulations of physicochemical characteristics of plasmas generated in different types of atmospheric-pressure discharges (pulsed streamer corona, gliding electric arc, dielectric barrier discharge, glow-discharge electrolysis, diaphragmatic discharge, and dc glow discharge) used to initiate various chemical processes in water solutions are analyzed. Typical reactor designs are considered. Data on the power supply characteristics, plasma electron parameters, gas temperatures, and densities of active particles in different types of discharges excited in different gases and their dependences on the external parameters of discharges are presented. The chemical composition of active particles formed in water is described. Possible mechanisms of production and loss of plasma particles are discussed.

Evolution of a plasma vortex in air

NASA Astrophysics Data System (ADS)

Tsai, Cheng-Mu; Chu, Hong-Yu

2016-01-01

We report the generation of a vortex-shaped plasma in air by using a capacitively coupled dielectric barrier discharge system. We show that a vortex-shaped plasma can be produced inside a helium gas vortex and is capable of propagating for 3 cm. The fluctuation of the plasma ring shows a scaling relation with the Reynolds number of the vortex. The transient discharge reveals the property of corona discharge, where the conducting channel within the gas vortex and the blur plasma emission are observed at each half voltage cycle.

Evolution of a plasma vortex in air.

PubMed

Tsai, Cheng-Mu; Chu, Hong-Yu

2016-01-01

We report the generation of a vortex-shaped plasma in air by using a capacitively coupled dielectric barrier discharge system. We show that a vortex-shaped plasma can be produced inside a helium gas vortex and is capable of propagating for 3 cm. The fluctuation of the plasma ring shows a scaling relation with the Reynolds number of the vortex. The transient discharge reveals the property of corona discharge, where the conducting channel within the gas vortex and the blur plasma emission are observed at each half voltage cycle.

Catheterized plasma X-ray source

DOEpatents

Derzon, Mark S.; Robinson, Alex; Galambos, Paul C.

2017-06-20

A radiation generator useful for medical applications, among others, is provided. The radiation generator includes a catheter; a plasma discharge chamber situated within a terminal portion of the catheter, a cathode and an anode positioned within the plasma discharge chamber and separated by a gap, and a high-voltage transmission line extensive through the interior of the catheter and terminating on the cathode and anode so as to deliver, in operation, one or more voltage pulses across the gap.

Generation of reactive species in atmospheric pressure dielectric barrier discharge with liquid water

NASA Astrophysics Data System (ADS)

Zelong, ZHANG; Jie, SHEN; Cheng, CHENG; Zimu, XU; Weidong, XIA

2018-04-01

Atmospheric pressure helium/water dielectric barrier discharge (DBD) plasma is used to investigate the generation of reactive species in a gas-liquid interface and in a liquid. The emission intensity of the reactive species is measured by optical emission spectroscopy (OES) with different discharge powers at the gas-liquid interface. Spectrophotometry is used to analyze the reactive species induced by the plasma in the liquid. The concentration of OH radicals reaches 2.2 μm after 3 min of discharge treatment. In addition, the concentration of primary long-lived reactive species such as H2O2, {{{{NO}}}3}- and O3 are measured based on plasma treatment time. After 5 min of discharge treatment, the concentration of H2O2, {{{{NO}}}3}-, and O3 increased from 0 mg · L-1 to 96 mg · L-1, 19.5 mg · L-1, and 3.5 mg · L-1, respectively. The water treated by plasma still contained a considerable concentration of reactive species after 6 h of storage. The results will contribute to optimizing the DBD plasma system for biological decontamination.

Studying the Generation Stage of a Plasma Jet in a Plasma Focus Discharge

NASA Astrophysics Data System (ADS)

Polukhin, S. N.; Gurei, A. E.; Nikulin, V. Ya.; Peregudova, E. N.; Silin, P. V.; Kharrasov, A. M.

2017-12-01

A dense compact plasmoid generated at the pinch collapse stage is revealed in a plasma focus discharge by laser optical methods. The initial size of the plasmoid is 1 mm, its electron density is more than 2 × 1019 cm-3, and the plasmoid propagates along the axis from the anode at an average velocity of more than 107 cm/s. A shock wave is generated in the residual argon plasma during the motion of the bunch, its density decreases to 1018 cm-3 at a distance of 3 cm from its place of generation, and the plasmoid expands by 3-5 times and almost merges together with the leading edge of the shock wave.

Fundamental experiment of ion thruster using ECR discharge

NASA Astrophysics Data System (ADS)

Yasui, Toshiaki; Kitayama, Jiro; Tahara, Hirokazu; Onoe, Ken-Ichi; Yoshikawa, Takao

A microwave ion thruster has the potential to overcome a lifetime problem of electric propulsion by eliminating electrodes. Two types of microwave ion thruster have been investigated to examine the operational characteristics. The one is the thruster using cavity-resonance microwave discharge, and the other is the thruster using Electron Cyclotron Resonance (ECR) discharge. Cavity-resonance microwave discharge produced plasmas by strong electric field in the resonant cavity and sustained plasmas at argon mass flow rates above 10 sccm. However, ECR discharge was capable of sustaining plasmas at lower mass flow rate, because ECR discharge efficiently produced plasmas by resonance absorption. From these generated microwave plasmas, ions were electrostatically extracted by two multiaperture grids. In ECR discharge, the maximum ion beam current of 75 mA and the highest mass utilization efficiency of 18.7% were achieved at a total extraction voltage of 950 V.

Pulsed Corona Discharge Generated By Marx Generator

NASA Astrophysics Data System (ADS)

Sretenovic, G. B.; Obradovic, B. M.; Kovacevic, V. V.; Kuraica, M. M.; Puric J.

2010-07-01

The pulsed plasma has a significant role in new environmental protection technologies. As a part of a pulsed corona system for pollution control applications, Marx type repetitive pulse generator was constructed and tested in arrangement with wire-plate corona reactor. We performed electrical measurements, and obtained voltage and current signals, and also power and energy delivered per pulse. Ozone formation by streamer plasma in air was chosen to monitor chemical activity of the pulsed corona discharge.

The effect of ethanol gas impurity on the discharge mode and discharge products of argon plasma jet at atmospheric pressure

NASA Astrophysics Data System (ADS)

Xia, Wenjie; Liu, Dingxin; Xu, Han; Wang, Xiaohua; Liu, Zhijie; Rong, Mingzhe; Kong, Michael G.

2018-05-01

Argon is a widely used working gas of plasmas, which is much cheaper than helium but on the other hand much more difficult to generate diffuse discharge at atmospheric pressure. In order to meet the application requirements, plenty of researches have been reported to facilitate the diffuse discharge happening for argon plasmas, and in this paper an approach of using ethanol gas (EtOH) impurity is investigated. The discharge characteristics of Ar + EtOH plasma jet are studied as a function of the applied voltage and the concentration of EtOH, from which the concentration of EtOH between ∼200 and ∼3300 parts per million (ppm) is determined necessary for the generation of diffuse discharge. Compared with the helium plasma jet in literature, it is deduced that the diffuse discharge is probably caused by the Penning ionization happening between the metastable argon and EtOH. The discharge products of Ar + EtOH (672 ppm) plasma jet are measured and the corresponding chemistry pathways are analyzed. About 20% of EtOH is decomposed via complex chemical reactions to form more than a dozen of neutral species, such as CH3CHO, CH3COOH, CO, H2O, and C n H2n+2 (n ≥ 3), and various kinds of ionic species, including C+, CH+, ArH+, {{{{O}}}2}-, CH3CH2O‑, etc.

Non-equilibrium plasma prevention of Schistosoma japonicum transmission

NASA Astrophysics Data System (ADS)

Wang, Xing-Quan; Wang, Feng-Peng; Chen, Wei; Huang, Jun; Bazaka, Kateryna; Ostrikov, Kostya (Ken)

2016-10-01

Schistosoma japonicum is a widespread human and animal parasite that causes intestinal and hepatosplenic schistosomiasis linked to colon, liver and bladder cancers, and anemia. Estimated 230 million people are currently infected with Schistosoma spp, with 779 million people at risk of contracting the parasite. Infection occurs when a host comes into contact with cercariae, a planktonic larval stage of the parasite, and can be prevented by inactivating the larvae, commonly by chemical treatment. We investigated the use of physical non-equilibrium plasma generated at atmospheric pressure using custom-made dielectric barrier discharge reactor to kill S. japonicum cercariae. Survival rate decreased with treatment time and applied power. Plasmas generated in O2 and air gas discharges were more effective in killing S. japonicum cercariae than that generated in He, which is directly related to the mechanism by which cercariae are inactivated. Reactive oxygen species, such as O atoms, abundant in O2 plasma and NO in air plasma play a major role in killing of S. japonicum cercariae via oxidation mechanisms. Similar level of efficacy is also shown for a gliding arc discharge plasma jet generated in ambient air, a system that may be more appropriate for scale-up and integration into existing water treatment processes.

Generation of anomalously energetic suprathermal electrons by an electron beam interacting with a nonuniform plasma

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sydorenko, D.; Kaganovich, I. D.; Chen, L.

Generation of anomalously energetic suprathermal electrons was observed in simulation of a high-voltage dc discharge with electron emission from the cathode. An electron beam produced by the emission interacts with the nonuniform plasma in the discharge via a two-stream instability. The energy transfer from the beam to the plasma electrons is ensured by the plasma nonuniformity. The electron beam excites plasma waves whose wavelength and phase speed gradually decrease towards anode. The waves with short wavelength near the anode accelerate plasma bulk electrons to suprathermal energies. The sheath near the anode reflects some of the accelerated electrons back into themore » plasma. These electrons travel through the plasma, reflect near the cathode, and enter the accelerating area again but with a higher energy than before. Such particles are accelerated to energies much higher than after the first acceleration. This mechanism plays a role in explaining earlier experimental observations of energetic suprathermal electrons in similar discharges.« less

Effects of gas temperature in the plasma layer on RONS generation in array-type dielectric barrier discharge at atmospheric pressure

NASA Astrophysics Data System (ADS)

Yoon, Sung-Young; Yi, Changho; Eom, Sangheum; Park, Seungil; Kim, Seong Bong; Ryu, Seungmin; Yoo, Suk Jae

2017-12-01

In this work, we studied the control of plasma-produced species under a fixed gas composition (i.e., ambient air) in a 10 kHz-driven array-type dielectric barrier atmospheric-pressure plasma discharge. Instead of the gas composition, only the gas velocity was controlled. Thus, the plasma-maintenance cost was considerably lower than methods such as external N2 or O2 injection. The plasma-produced species were monitored using Fourier transformed infrared spectroscopy. The discharge properties were measured using a voltage probe, current probe, infrared camera, and optical emission spectroscopy. The results showed that the major plasma products largely depend on the gas temperature in the plasma discharge layer. The gas temperature in the plasma discharge layer was significantly different to the temperature of the ceramic adjacent to the plasma discharge layer, even in the small discharge power density of ˜15 W/cm2 or ˜100 W/cm3. Because the vibrational excitation of N2 was suppressed by the higher gas flow, the major plasma-produced species shifted from NOx in low flow to O3 in high flow.

Directional mass transport in an atmospheric pressure surface barrier discharge.

PubMed

Dickenson, A; Morabit, Y; Hasan, M I; Walsh, J L

2017-10-25

In an atmospheric pressure surface barrier discharge the inherent physical separation between the plasma generation region and downstream point of application reduces the flux of reactive chemical species reaching the sample, potentially limiting application efficacy. This contribution explores the impact of manipulating the phase angle of the applied voltage to exert a level of control over the electrohydrodynamic forces generated by the plasma. As these forces produce a convective flow which is the primary mechanism of species transport, the technique facilitates the targeted delivery of reactive species to a downstream point without compromising the underpinning species generation mechanisms. Particle Imaging Velocimetry measurements are used to demonstrate that a phase shift between sinusoidal voltages applied to adjacent electrodes in a surface barrier discharge results in a significant deviation in the direction of the plasma induced gas flow. Using a two-dimensional numerical air plasma model, it is shown that the phase shift impacts the spatial distribution of the deposited charge on the dielectric surface between the adjacent electrodes. The modified surface charge distribution reduces the propagation length of the discharge ignited on the lagging electrode, causing an imbalance in the generated forces and consequently a variation in the direction of the resulting gas flow.

Study of ultrasound-assisted radio-frequency plasma discharges in n-dodecane

NASA Astrophysics Data System (ADS)

Camerotto, Elisabeth; De Schepper, Peter; Nikiforov, Anton Y.; Brems, Steven; Shamiryan, Denis; Boullart, Werner; Leys, Christophe; De Gendt, Stefan

2012-10-01

This paper investigates the generation of a stable plasma phase in a liquid hydrocarbon (n-dodecane) by means of ultrasound (US) and radio-frequency (RF) or electromagnetic radiation. It is demonstrated for the first time that ultrasonic aided RF plasma discharges can be generated in a liquid. Plasma discharges are obtained for different gas mixtures at a pressure of 12 kPa and at low ignition powers (100 W for RF and 2.4 W cm-2 for US). Direct carbon deposition from the liquid precursor on Cu, Ni, SiO2 and Si substrates has been obtained and no apparent compositional or structural difference among the substrate materials was observed. Characterization of the deposited solid phase revealed an amorphous structure. In addition, structural changes in the liquid precursor after plasma treatment have been analysed. Optical emission spectroscopy (OES) allowed the estimation of several plasma characteristic temperatures. The plasma excitation temperature was estimated to be about 2.3-2.4 eV. The rotational and vibrational temperatures of the discharge in n-dodecane with Ar as a feed gas were 1400 K and 6500 K, respectively. In Ar/O2 plasma, an increased rotational (1630 K) and vibrational temperature (7200 K) were obtained.

Experimental study of atmospheric-pressure micro-plasmas for the ambient sampling of conductive materials

NASA Astrophysics Data System (ADS)

Duan, Zhengchao; He, Feng; Si, Xinlu; Bradley, James W.; Ouyang, Jiting

2018-02-01

Conductive solid material sampling by micro-plasma under ambient atmosphere was studied experimentally. A high-voltage pulse generator was utilized to drive discharge between a tungsten needle and metal samples. The effects of pulse width on discharge, micro-plasma and sampling were investigated. The electrical results show that two discharge current pulses can be formed in one voltage pulse. The duration of the first current pulse is of the order of 100 ns. The duration of the second current pulse depends on the width of the voltage pulse. The electrical results also show that arc micro-plasma was generated during both current pulses. The results of the emission spectra of different sampled materials indicate that the relative emission intensity of elemental metal ions will increase with pulse width. The excitation temperature and electron density of the arc micro-plasmas increase with the voltage pulse width, which contributes to the increase of relative emission intensity of metal ions. The optical images and energy dispersive spectroscopy results of the sampling spots on metal surfaces indicate that discharge with a short voltage pulse can generate a small sputtering crater.

The cold and atmospheric-pressure air surface barrier discharge plasma for large-area sterilization applications

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang Dacheng; Department of Aeronautics, Fujian Key Laboratory for Plasma and Magnetic Resonance, School of Physics and Mechanical and Electrical Engineering, Xiamen University, Xiamen, Fujian 361005; Zhao Di

2011-04-18

This letter reports a stable air surface barrier discharge device for large-area sterilization applications at room temperature. This design may result in visually uniform plasmas with the electrode area scaled up (or down) to the required size. A comparison for the survival rates of Escherichia coli from air, N{sub 2} and O{sub 2} surface barrier discharge plasmas is presented, and the air surface plasma consisting of strong filamentary discharges can efficiently kill Escherichia coli. Optical emission measurements indicate that reactive species such as O and OH generated in the room temperature air plasmas play a significant role in the sterilizationmore » process.« less

Study of Plasma Flows Generated in Plasma Focus Discharge in Different Regimes of Working Gas Filling

NASA Astrophysics Data System (ADS)

Voitenko, D. A.; Ananyev, S. S.; Astapenko, G. I.; Basilaia, A. D.; Markolia, A. I.; Mitrofanov, K. N.; Myalton, V. V.; Timoshenko, A. P.; Kharrasov, A. M.; Krauz, V. I.

2017-12-01

Results are presented from experimental studies of the plasma flows generated in the KPF-4 Phoenix Mather-type plasma focus device (Sukhum Physical Technical Institute). In order to study how the formation and dynamics of the plasma flow depend on the initial distribution of the working gas, a system of pulsed gas puffing into the discharge volume was developed. The system allows one to create profiled gas distributions, including those with a reduced gas density in the region of plasma flow propagation. Results of measurements of the magnetic field, flow profile, and flow deceleration dynamics at different initial distributions of the gas pressure are presented.

Comparison of electrical and optical characteristics in gas-phase and gas-liquid phase discharges

DOE Office of Scientific and Technical Information (OSTI.GOV)

Qazi, H. I. A.; Li, He-Ping, E-mail: liheping@tsinghua.edu.cn; Zhang, Xiao-Fei

This paper presents an AC-excited argon discharge generated using a gas-liquid (two-phase) hybrid plasma reactor, which mainly consists of a powered needle electrode enclosed in a conical quartz tube and grounded deionized water electrode. The discharges in the gas-phase, as well as in the two-phase, exhibit two discharge modes, i.e., the low current glow-like diffuse mode and the high current streamer-like constrict mode, with a mode transition, which exhibits a negative resistance of the discharges. The optical emission spectral analysis shows that the stronger diffusion of the water vapor into the discharge region in the two-phase discharges boosts up themore » generation of OH (A–X) radicals, and consequently, leads to a higher rotational temperature in the water-phase plasma plume than that of the gas-phase discharges. Both the increase of the power input and the decrease of the argon flow rate result in the increase of the rotational temperature in the plasma plume of the water-phase discharge. The stable two-phase discharges with a long plasma plume in the water-phase under a low power input and gas flow rate may show a promising prospect for the degradation of organic pollutants, e.g., printing and dyeing wastewater, in the field of environmental protection.« less

Spontaneous Generation of a Sheared Plasma Rotation in a Field-Reversed θ-Pinch Discharge

NASA Astrophysics Data System (ADS)

Omelchenko, Y. A.; Karimabadi, H.

2012-08-01

By conducting two-dimensional hybrid simulations of an infinitely long field-reversed θ-pinch discharge we discover a new type of plasma rotation, which rapidly develops at the plasma edge in the ion diamagnetic direction due to the self-consistent generation of a Hall-driven radial electric field. This effect is different from the previously identified end-shorting and particle-loss mechanisms. We also demonstrate flutelike perturbations frequently inferred in experiments and show that in the absence of axial contraction effects they may quickly alter the toroidal symmetry of the plasma.

Beam heated linear theta-pinch device for producing hot plasmas

DOEpatents

Bohachevsky, Ihor O.

1981-01-01

A device for producing hot plasmas comprising a single turn theta-pinch coil, a fast discharge capacitor bank connected to the coil, a fuel element disposed along the center axis of the coil, a predetermined gas disposed within the theta-pinch coil, and a high power photon, electron or ion beam generator concentrically aligned to the theta-pinch coil. Discharge of the capacitor bank generates a cylindrical plasma sheath within the theta-pinch coil which heats the outer layer of the fuel element to form a fuel element plasma layer. The beam deposits energy in either the cylindrical plasma sheath or the fuel element plasma layer to assist the implosion of the fuel element to produce a hot plasma.

Collective phenomena in volume and surface barrier discharges

NASA Astrophysics Data System (ADS)

Kogelschatz, U.

2010-11-01

Barrier discharges are increasingly used as a cost-effective configuration to produce non-equilibrium plasmas at atmospheric pressure. This way, copious amounts of electrons, ions, free radicals and excited species can be generated without significant heating of the background gas. In most applications the barrier is made of dielectric material. Major applications utilizing mainly dielectric barriers include ozone generation, surface cleaning and modification, polymer and textile treatment, sterilization, pollution control, CO2 lasers, excimer lamps, plasma display panels (flat TV screens). More recent research efforts are devoted to biomedical applications and to plasma actuators for flow control. Sinusoidal feeding voltages at various frequencies as well as pulsed excitation schemes are used. Volume as well as surface barrier discharges can exist in the form of filamentary, regularly patterned or diffuse, laterally homogeneous discharges. The physical effects leading to collective phenomena in volume and surface barrier discharges are discussed in detail. Special attention is paid to self-organization of current filaments and pattern formation. Major similarities of the two types of barrier discharges are elaborated.

Demonstration of multi-generational growth of tungsten nanoparticles in hydrogen plasma using in situ laser extinction method

NASA Astrophysics Data System (ADS)

Ouaras, K.; Lombardi, G.; Hassouni, K.

2018-03-01

For the first time, we demonstrate that tungsten (W) nanoparticles (NPs) are created when a tungsten target is exposed to low-pressure, high density hydrogen plasma. The plasma was generated using a novel dual plasma system combining a microwave discharge and a pulsed direct-current (DC) discharge. The tungsten surface originates in the multi-generational formation of a significant population of 30-70 nm diameter particles when the W cathode is biased at ~  -1 kV and submitted to ~1020 m2 s-1 H+/H2+ /H3+ ions flux. The evidenced NPs formation should be taking into account as one of the consequence of the plasma surface interaction outcomes, especially for fusion applications.

Demonstration of plasma start-up by Coaxial Helicity Injection

NASA Astrophysics Data System (ADS)

Raman, Roger

2003-10-01

Experimental results on the first successful transfer of a Coaxial-Helicity-Injection- (CHI)-produced discharge to inductive operation are reported. CHI assisted plasma start-up is more robust than inductive-only operation and reduces volt-seconds consumption. After hand-off for inductive operation, the initial 100 kA of CHI-produced current drops to 44 kA, then ramps up to 180 kA, using only 30 mVs, more than 30induction alone. Coupling a CHI-produced discharge to induction from a pre-charged central solenoid has produced record plasma currents of 265kA in HIT-II. CHI discharges can also be generated while the central transformer is in the process of being pre-charged, during which period it induces a negative loop voltage on the CHI discharge. Such capability is believed to be important for a short pulse burning plasma experiment that could contain a solenoid. In the latest results, which improve upon the earlier work (Raman et. al., Phys. Rev. Lett., 90, (2003) 075005-1), no transient coil currents are necessary for the CHI produced closed flux generation. This is particularly important for a reactor in which the poloidal field coils would be located outside blanket structures. Three important results are reported. First, CHI is shown to produce closed flux plasma. Second, it is shown that electrode-based CHI plasmas can be sufficiently clean for fusion research purposes. Finally, it is shown that CHI discharges, in addition to generating useful startup current, improve the performance of inductive discharges. This work was motivated by earlier experiments on HIT-II and NSTX that showed coupling of the inductive drive to the external CHI power supply circuit, instead of to the main plasma discharge. These important results were obtained on the HIT-II spherical torus experiment (R/a of 0.3/0.2m, elongation of 1.5).

Experimental Investigation of Pseudospark generated electron beam

NASA Astrophysics Data System (ADS)

Kumar, Niraj; Verma, D. K.; Prajapati, J.; Kumar, M.; Meena, B. L.; Tyagi, M. S.; Srivastava, V.; Pal, U. N.

2012-11-01

The pseudospark (PS) discharge is, however, more recently recognized as a different type of discharge which is capable of generating electron beams with the highest combined current density and brightness of any known type of electron source. PS discharge is a specific type of gas discharge, which operates on the left-hand side of the hollow cathode analogy to the Paschen curve with axially symmetric parallel electrodes and central holes on the electrodes. The PS discharge generated electron beam has tremendous applications in plasma filled microwave sources where normal material cathode cannot be used. Analysis of the electron beam profile has been carried out experimentally for different applied voltages. The investigation has been done at different axial and radial location inside the drift tube in argon atmosphere. This paper represents experimentally derived axial and radial variation of the beam current inside the plasma filled drift tube of PS discharge based plasma cathode electron (PCE) gun. With the help of current density estimation the focusing and defocusing point of electron beam in axial direction can be analyzed. It has been further confirmed the successful propagation of electron beam in confined manner without any assistance of external magnetic field.

Characteristics of back corona discharge in a honeycomb catalyst and its application for treatment of volatile organic compounds.

PubMed

Feng, Fada; Zheng, Yanyan; Shen, Xinjun; Zheng, Qinzhen; Dai, Shaolong; Zhang, Xuming; Huang, Yifan; Liu, Zhen; Yan, Keping

2015-06-02

The main technical challenges for the treatment of volatile organic compounds (VOCs) with plasma-assisted catalysis in industrial applications are large volume plasma generation under atmospheric pressure, byproduct control, and aerosol collection. To solve these problems, a back corona discharge (BCD) configuration has been designed to evenly generate nonthermal plasma in a honeycomb catalyst. Voltage-current curves, discharge images, and emission spectra have been used to characterize the plasma. Grade particle collection results and flow field visualization in the discharge zones show not only that the particles can be collected efficiently, but also that the pressure drop of the catalyst layer is relatively low. A three-stage plasma-assisted catalysis system, comprising a dielectric barrier discharge (DBD) stage, BCD stage, and catalyst stage, was built to evaluate toluene treatment performance by BCD. The ozone analysis results indicate that BCD enhances the ozone decomposition by collecting aerosols and protecting the Ag-Mn-O catalyst downstream from aerosol contamination. The GC and FTIR results show that BCD contributes to toluene removal, especially when the specific energy input is low, and the total removal efficiency reaches almost 100%. Furthermore, this removal results in the emission of fewer byproducts.

Atmospheric-pressure diffuse dielectric barrier discharges in Ar/O2 gas mixture using 200 kHz/13.56 MHz dual frequency excitation

NASA Astrophysics Data System (ADS)

Liu, Y.; Starostin, S. A.; Peeters, F. J. J.; van de Sanden, M. C. M.; de Vries, H. W.

2018-03-01

Atmospheric-pressure diffuse dielectric barrier discharges (DBDs) were obtained in Ar/O2 gas mixture using dual-frequency (DF) excitation at 200 kHz low frequency (LF) and 13.56 MHz radio frequency (RF). The excitation dynamics and the plasma generation mechanism were studied by means of electrical characterization and phase resolved optical emission spectroscopy (PROES). The DF excitation results in a time-varying electric field which is determined by the total LF and RF gas voltage and the spatial ion distribution which only responds to the LF component. By tuning the amplitude ratio of the superimposed LF and RF signals, the effect of each frequency component on the DF discharge mechanism was analysed. The LF excitation results in a transient plasma with the formation of an electrode sheath and therefore a pronounced excitation near the substrate. The RF oscillation allows the electron trapping in the gas gap and helps to improve the plasma uniformity by contributing to the pre-ionization and by controlling the discharge development. The possibility of temporally modifying the electric field and thus the plasma generation mechanism in the DF discharge exhibits potential applications in plasma-assisted surface processing and plasma-assisted gas phase chemical conversion.

Characteristics of soft x-ray spectra from ultra-fast micro-capillary discharge plasmas

NASA Astrophysics Data System (ADS)

Li, Jing; Avaria, Gonzalo; Shlyaptsev, Vyacheslav; Tomasel, Fernando; Grisham, Michael; Dawson, Quincy; Rocca, Jorge; NSF CenterExtreme Ultraviolet Science; Technology Collaboration

2013-10-01

The efficient generation of high aspect ratio (e.g. 300:1) plasma columns ionized to very high degrees of ionization (e.g. Ni-like Xenon) by an ultrafast current pulses of moderate amplitude in micro-capillary channels is of interest for fundamental plasma studies and for applications such as the generation of discharge-pumped soft x-ray lasers. Spectra and simulations for plasmas generated in 500 um alumina capillary discharges driven by 35-40 kA current pulses with 4 ns rise time were obtained in Xenon and Neon discharges. The first shows the presence of lines corresponding to ionization stages up to Fe-like Xe. The latter show that Al impurities from the walls and Si (from injected SiH4) are ionized to the H-like and He-like stages. He-like spectra containing the resonance line significantly broaden by opacity, the intercombination line, and Li-like satellites are analyzed and modeled. For Xenon discharges, the spectral lines from the Ni-like transitions the 3d94d(3/2, 3/2)J=0 to the 3d94p(5/2, 3/2)J=1 and to 3d94p(3/2, 1/2)J=1 are observed at gas pressures up to 2.0 Torr. Work supported by NSF Award PHY-1004295.

Reaction of Cl- ions in electrolyte solution induced electrical discharge plasma in the presence of argon fine bubbles

NASA Astrophysics Data System (ADS)

Hayashi, Yui; Takada, Noriharu; Wahyudiono, Kanda, Hideki; Goto, Motonobu

2017-05-01

Active chlorine species such as chlorine molecules and hypochlorous acid have been known as high performance sanitizers. They would act more reactive on chemical and biological substances when an electrical discharge was introduced in water containing an electrolyte substance. Here, the reaction of chloride (Cl-) ions were examined by introducing of a pulsed discharge plasma in sodium chloride (NaCl) solution as an electrolyte solution at room temperature. The results show that a large electrical current generated by the pulsed discharge plasma affected the reaction of Cl- ions to result available chlorine. The reaction pathway for available chlorine production was assumed similar with the reaction pathway as electrolysis. A pulsed discharge plasma in NaCl solution in the presence of argon (Ar) fine bubbles exhibited intense emissions and high electron density compared to when no Ar fine bubbles were introduced. At these conditions, the dissociation reaction rate of water increased drastically leads to the formation of 0 atoms. As a result, the reaction of Cl- ions and the available chlorine generation were also increased.

Modeling of plasma chemical processes in the artificial ionized layer in the upper atmosphere by the nanosecond corona discharge

NASA Astrophysics Data System (ADS)

Vikharev, A. L.; Gorbachev, A. M.; Ivanov, O. A.; Kolisko, A. L.; Litvak, A. G.

1993-08-01

The plasma chemical processes in the corona discharge formed in air by a series of high voltage pulses of nanosecond duration are investigated experimentally. The experimental conditions (reduced electric field, duration and repetition frequency of the pulses, gas pressure in the chamber) modeled the regime of creation of the artificial ionized layer (AIL) in the upper atmosphere by a nanosecond microwave discharge. It was found that in a nanosecond microwave discharge predominantly generation of ozone occurs, and that the production of nitrogen dioxide is not large. The energy expenditures for the generation of one O 3 molecule were about 15 eV. On the basis of the experimental results the prognosis of the efficiency of ozone generation in AIL was made.

FAST TRACK COMMUNICATION: Asymmetric surface barrier discharge plasma driven by pulsed 13.56 MHz power in atmospheric pressure air

NASA Astrophysics Data System (ADS)

Dedrick, J.; Boswell, R. W.; Charles, C.

2010-09-01

Barrier discharges are a proven method of generating plasmas at high pressures, having applications in industrial processing, materials science and aerodynamics. In this paper, we present new measurements of an asymmetric surface barrier discharge plasma driven by pulsed radio frequency (rf 13.56 MHz) power in atmospheric pressure air. The voltage, current and optical emission of the discharge are measured temporally using 2.4 kVp-p (peak to peak) 13.56 MHz rf pulses, 20 µs in duration. The results exhibit different characteristics to plasma actuators, which have similar discharge geometry but are typically driven at frequencies of up to about 10 kHz. However, the electrical measurements are similar to some other atmospheric pressure, rf capacitively coupled discharge systems with symmetric electrode configurations and different feed gases.

Kinetic study on non-thermal volumetric plasma decay in the early afterglow of air discharge generated by a short pulse microwave or laser

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yang, Wei, E-mail: yangwei861212@126.com; Zhou, Qianhong; Dong, Zhiwei

This paper reports a kinetic study on non-thermal plasma decay in the early afterglow of air discharge generated by short pulse microwave or laser. A global self-consistent model is based on the particle balance of complex plasma chemistry, electron energy equation, and gas thermal balance equation. Electron-ion Coulomb collision is included in the steady state Boltzmann equation solver to accurately describe the electron mobility and other transport coefficients. The model is used to simulate the afterglow of microsecond to nanosecond pulse microwave discharge in N{sub 2}, O{sub 2}, and air, as well as femtosecond laser filament discharge in dry andmore » humid air. The simulated results for electron density decay are in quantitative agreement with the available measured ones. The evolution of plasma decay under an external electric field is also investigated, and the effect of gas heating is considered. The underlying mechanism of plasma density decay is unveiled through the above kinetic modeling.« less

Large area atmospheric-pressure plasma jet

DOEpatents

Selwyn, Gary S.; Henins, Ivars; Babayan, Steve E.; Hicks, Robert F.

2001-01-01

Large area atmospheric-pressure plasma jet. A plasma discharge that can be operated at atmospheric pressure and near room temperature using 13.56 MHz rf power is described. Unlike plasma torches, the discharge produces a gas-phase effluent no hotter than 250.degree. C. at an applied power of about 300 W, and shows distinct non-thermal characteristics. In the simplest design, two planar, parallel electrodes are employed to generate a plasma in the volume therebetween. A "jet" of long-lived metastable and reactive species that are capable of rapidly cleaning or etching metals and other materials is generated which extends up to 8 in. beyond the open end of the electrodes. Films and coatings may also be removed by these species. Arcing is prevented in the apparatus by using gas mixtures containing He, which limits ionization, by using high flow velocities, and by properly spacing the rf-powered electrode. Because of the atmospheric pressure operation, there is a negligible density of ions surviving for a sufficiently long distance beyond the active plasma discharge to bombard a workpiece, unlike the situation for low-pressure plasma sources and conventional plasma processing methods.

Atmospheric-pressure plasma jet

DOEpatents

Selwyn, Gary S.

1999-01-01

Atmospheric-pressure plasma jet. A .gamma.-mode, resonant-cavity plasma discharge that can be operated at atmospheric pressure and near room temperature using 13.56 MHz rf power is described. Unlike plasma torches, the discharge produces a gas-phase effluent no hotter than 250.degree. C. at an applied power of about 300 W, and shows distinct non-thermal characteristics. In the simplest design, two concentric cylindrical electrodes are employed to generate a plasma in the annular region therebetween. A "jet" of long-lived metastable and reactive species that are capable of rapidly cleaning or etching metals and other materials is generated which extends up to 8 in. beyond the open end of the electrodes. Films and coatings may also be removed by these species. Arcing is prevented in the apparatus by using gas mixtures containing He, which limits ionization, by using high flow velocities, and by properly shaping the rf-powered electrode. Because of the atmospheric pressure operation, no ions survive for a sufficiently long distance beyond the active plasma discharge to bombard a workpiece, unlike low-pressure plasma sources and conventional plasma processing methods.

An investigation of transient pressure and plasma properties in a pinched plasma column. M.S. Thesis

NASA Technical Reports Server (NTRS)

Stover, E. K.; York, T. M.

1971-01-01

The transient pinched plasma column generated in a linear Z-pinch was studied experimentally and analytically. The plasma column was investigated experimentally with the following plasma diagnostics: a special rapid response pressure transducer, a magnetic field probe, a voltage probe and discharge luminosity. Axial pressure profiles on the discharge chamber axis were used to identify three characteristic regions of plasma column behavior; they were in temporal sequence: strong axial pressure asymmetry noted early in plasma column lifetime followed by plasma heating in which there is a rapid rise in static pressure and a slight decrease static pressure before plasma column breakup. Plasma column lifetime was approximately 5 microseconds. The axial pressure asymmetry was attributed to nonsimultaneous pinching of the imploding current sheet along the discharge chamber axis. The rapid heating is attributed in part to viscous effects introduced by radial gradients in the axial streaming velocity. Turbulent heating arising from discharge current excitation of the ion acoustic wave instability is also considered a possible heating mechanism.

A large-area diffuse air discharge plasma excited by nanosecond pulse under a double hexagon needle-array electrode.

PubMed

Liu, Zhi-Jie; Wang, Wen-Chun; Yang, De-Zheng; Wang, Sen; Zhang, Shuai; Tang, Kai; Jiang, Peng-Chao

2014-01-01

A large-area diffuse air discharge plasma excited by bipolar nanosecond pulse is generated under a double hexagon needle-array electrode at atmospheric pressure. The images of the diffuse discharge, electric characteristics, and the optical emission spectra emitted from the diffuse air discharge plasma are obtained. Based on the waveforms of pulse voltage and current, the power consumption, and the power density of the diffuse air discharge plasma are investigated under different pulse peak voltages. The electron density and the electron temperature of the diffuse plasma are estimated to be approximately 1.42×10(11) cm(-3) and 4.4 eV, respectively. The optical emission spectra are arranged to determine the rotational and vibrational temperatures by comparing experimental with simulated spectra. Meanwhile, the rotational and vibrational temperatures of the diffuse discharge plasma are also discussed under different pulse peak voltages and pulse repetition rates, respectively. In addition, the diffuse air discharge plasma can form an area of about 70×50 mm(2) on the surface of dielectric layer and can be scaled up to the required size. Crown Copyright © 2013. Published by Elsevier B.V. All rights reserved.

Electron cyclotron plasma startup in the GDT experiment

NASA Astrophysics Data System (ADS)

Yakovlev, D. V.; Shalashov, A. G.; Gospodchikov, E. D.; Solomakhin, A. L.; Savkin, V. Ya.; Bagryansky, P. A.

2017-01-01

We report on a new plasma startup scenario in the gas dynamic trap (GDT) magnetic mirror device. The primary 5 MW neutral beam injection (NBI) plasma heating system fires into a sufficiently dense plasma target (‘seed plasma’), which is commonly supplied by an arc plasma generator. In the reported experiments, a different approach to seed plasma generation is explored. One of the channels of the electron cyclotron resonance (ECR) heating system is used to ionize the neutral gas and build up the density of plasma to a level suitable for NBI capture. After a short transition of approximately 1 ms the discharge becomes essentially similar to a standard one initiated by the plasma gun. This paper presents the discharge scenario and experimental data on the seed plasma evolution during ECRH, along with the dependencies on incident microwave power, magnetic configuration and pressure of a neutral gas. The characteristics of the consequent high-power NBI discharge are studied and differences from the conventional scenario are discussed. A theoretical model describing the ECR breakdown and the seed plasma accumulation in a large-scale mirror trap is developed on the basis of the GDT experiment.

A study of the glow discharge plasma jet of the novel Hamburger-electrode

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Wenzheng, E-mail: wzhliu@bjtu.edu.cn; Ma, Chuanlong, E-mail: 15121452@bjtu.edu.cn; Yang, Xiao

2016-08-15

To generate atmospheric pressure glow discharge plasma jets (APGDPJs), a novel Hamburger-electrode was proposed. Through the study on electric field distributions, flow field distributions, and characteristics of the discharge and jet, we found that adopting the mode of dielectric barrier discharge with non-uniform thickness of dielectric, it was easy to form the strong electric field areas which were conducive to generate discharge and electric field distributions with large electric field intensity in the narrow gap and weak electric field intensity in the wide gap that were not inclined to form a filament discharge. Using the structure of evenly distributed innermore » electrodes, it was easy to weaken the pressure of strong electric field areas and form flow field distributions which is beneficial for taking out the high density charged particles and generating APGDPJs. Stable APGDPJs in nitrogen with 3.5 mm in diameter and 9 mm in length were formed by using the novel Hamburger-electrode.« less

Solenoid-free plasma startup in NSTX using transient CHI

NASA Astrophysics Data System (ADS)

Raman, R.; Jarboe, T. R.; Mueller, D.; Nelson, B. A.; Bell, M. G.; Bell, R.; Gates, D.; Gerhardt, S.; Hosea, J.; Kaita, R.; Kugel, H.; LeBlanc, B.; Maingi, R.; Maqueda, R.; Menard, J.; Nagata, M.; Ono, M.; Paul, S.; Roquemore, L.; Sabbagh, S.; Soukhanovskii, V.; Taylor, G.

2009-06-01

Experiments in NSTX have now demonstrated the coupling of toroidal plasmas produced by the technique of coaxial helicity injection (CHI) to inductive sustainment and ramp-up of the toroidal plasma current. In these discharges, the central Ohmic transformer was used to apply an inductive loop voltage to discharges with a toroidal current of about 100 kA created by CHI. The coupled discharges have ramped up to >700 kA and transitioned into an H-mode demonstrating compatibility of this startup method with conventional operation. The electron temperature in the coupled discharges reached over 800 eV and the resulting plasma had low inductance, which is preferred for long-pulse high-performance discharges. These results from NSTX in combination with the previously obtained record 160 kA non-inductively generated startup currents in an ST or tokamak in NSTX demonstrate that CHI is a viable solenoid-free plasma startup method for future STs and tokamaks.

Low Cost, Efficient Microcavity Plasma Ozone Generation for Water Remediation and Air Purification

DTIC Science & Technology

2012-06-01

Eliasson, and M. Hirth, “ Ozone Generation from Oxygen and Air: Discharge Physics and Reaction Mechanisms,” Ozone Sci. and Eng., vol. 10, pp. 367-378...Phase I Final Report: Low Cost, Efficient Microcavity Plasma Ozone Generation for Water Remediation and Air Purification...Contract Number: FA9550-11-C-0087 June 2012 Low Cost, Efficient Microcavity Plasma Ozone Generation for Water Remediation

Effects of Non-Equilibrium Plasmas on Low-Pressure, Premixed Flames. Part 1: CH* Chemiluminescence, Temperature, and OH

DTIC Science & Technology

2018-01-16

1    Effects of Non -Equilibrium Plasmas on Low-Pressure, Premixed Flames. Part 1: CH* Chemiluminescence, Temperature, and OH Ting Li, Igor V...investigate the effects of nanosecond, repetitively-pulsed, non -equilibrium plasma discharges on laminar, low-pressure, premixed burner-stabilized hydrogen/O2...sources, both of which generate uniform, low-temperature, volumetric, non -equilibrium plasma discharges, are used to study changes in

Laser-Based Optical System for Reactive Radical Concentration Measurements in Plasmas and Flames

DTIC Science & Technology

2006-08-01

role of different plasma components in chain propagation support: (1) and (2) - corona plasma generators with high-voltage multiple needle electrodes ; (3...H20 2) and HCN. Measurements in Gliding Arc, Dielectric Barrier Discharge and Pulsed Corona Plasma systems and in flame and flow reactor systems are...discharges operating in air with iron electrodes - 260V.35 Using visual quantification from high speed camera arc images, the approximate thickness of

Investigation of flame structure in plasma-assisted turbulent premixed methane-air flame

NASA Astrophysics Data System (ADS)

Hualei, ZHANG; Liming, HE; Jinlu, YU; Wentao, QI; Gaocheng, CHEN

2018-02-01

The mechanism of plasma-assisted combustion at increasing discharge voltage is investigated in detail at two distinctive system schemes (pretreatment of reactants and direct in situ discharge). OH-planar laser-induced fluorescence (PLIF) technique is used to diagnose the turbulent structure methane-air flame, and the experimental apparatus consists of dump burner, plasma-generating system, gas supply system and OH-PLIF system. Results have shown that the effect of pretreatment of reactants on flame can be categorized into three regimes: regime I for voltage lower than 6.6 kV; regime II for voltage between 6.6 and 11.1 kV; and regime III for voltage between 11.1 and 12.5 kV. In regime I, aerodynamic effect and slower oxidation of higher hydrocarbons generated around the inner electrode tip plays a dominate role, while in regime III, the temperature rising effect will probably superimpose on the chemical effect and amplify it. For wire-cylinder dielectric barrier discharge reactor with spatially uneven electric field, the amount of radicals and hydrocarbons are decreased monotonically in radial direction which affects the flame shape. With regard to in situ plasma discharge in flames, the discharge pattern changes from streamer type to glow type. Compared with the case of reactants pretreatment, the flame propagates further in the upstream direction. In the discharge region, the OH intensity is highest for in situ plasma assisted combustion, indicating that the plasma energy is coupled into flame reaction zone.

Absorption of a laser light pulse in a dense plasma.

NASA Technical Reports Server (NTRS)

Mehlman-Balloffet, G.

1973-01-01

An experimental study of the absorption of a laser light pulse in a transient, high-density, high-temperature plasma is presented. The plasma is generated around a metallic anode tip by a fast capacitive discharge occurring in vacuum. The amount of transmitted light is measured for plasmas made of different metallic ions in the regions of the discharge of high electronic density. Variation of the transmission during the laser pulse is also recorded. Plasma electrons are considered responsible for the very high absorption observed.

High-frequency underwater plasma discharge application in antibacterial activity

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ahmed, M. W.; Choi, S.; Lyakhov, K.

Plasma discharge is a novel disinfection and effectual inactivation approach to treat microorganisms in aqueous systems. Inactivation of Gram-negative Escherichia coli (E. coli) by generating high-frequency, high-voltage, oxygen (O{sub 2}) injected and hydrogen peroxide (H{sub 2}O{sub 2}) added discharge in water was achieved. The effect of H{sub 2}O{sub 2} dose and oxygen injection rate on electrical characteristics of discharge and E. coli disinfection has been reported. Microbial log reduction dependent on H{sub 2}O{sub 2} addition with O{sub 2} injection was observed. The time variation of the inactivation efficiency quantified by the log reduction of the initial E. coli population onmore » the basis of optical density measurement was reported. The analysis of emission spectrum recorded after discharge occurrence illustrated the formation of oxidant species (OH{sup •}, H, and O). Interestingly, the results demonstrated that O{sub 2} injected and H{sub 2}O{sub 2} added, underwater plasma discharge had fabulous impact on the E. coli sterilization. The oxygen injection notably reduced the voltage needed for generating breakdown in flowing water and escalated the power of discharge pulses. No impact of hydrogen peroxide addition on breakdown voltage was observed. A significant role of oxidant species in bacterial inactivation also has been identified. Furthermore the E. coli survivability in plasma treated water with oxygen injection and hydrogen peroxide addition drastically reduced to zero. The time course study also showed that the retardant effect on E. coli colony multiplication in plasma treated water was favorable, observed after long time. High-frequency underwater plasma discharge based biological applications is technically relevant and would act as baseline data for the development of novel antibacterial processing strategies.« less

High-frequency underwater plasma discharge application in antibacterial activity

NASA Astrophysics Data System (ADS)

Ahmed, M. W.; Choi, S.; Lyakhov, K.; Shaislamov, U.; Mongre, R. K.; Jeong, D. K.; Suresh, R.; Lee, H. J.

2017-03-01

Plasma discharge is a novel disinfection and effectual inactivation approach to treat microorganisms in aqueous systems. Inactivation of Gram-negative Escherichia coli ( E. coli) by generating high-frequency, high-voltage, oxygen (O2) injected and hydrogen peroxide (H2O2) added discharge in water was achieved. The effect of H2O2 dose and oxygen injection rate on electrical characteristics of discharge and E. coli disinfection has been reported. Microbial log reduction dependent on H2O2 addition with O2 injection was observed. The time variation of the inactivation efficiency quantified by the log reduction of the initial E. coli population on the basis of optical density measurement was reported. The analysis of emission spectrum recorded after discharge occurrence illustrated the formation of oxidant species (OH•, H, and O). Interestingly, the results demonstrated that O2 injected and H2O2 added, underwater plasma discharge had fabulous impact on the E. coli sterilization. The oxygen injection notably reduced the voltage needed for generating breakdown in flowing water and escalated the power of discharge pulses. No impact of hydrogen peroxide addition on breakdown voltage was observed. A significant role of oxidant species in bacterial inactivation also has been identified. Furthermore the E. coli survivability in plasma treated water with oxygen injection and hydrogen peroxide addition drastically reduced to zero. The time course study also showed that the retardant effect on E. coli colony multiplication in plasma treated water was favorable, observed after long time. High-frequency underwater plasma discharge based biological applications is technically relevant and would act as baseline data for the development of novel antibacterial processing strategies.

The component content of active particles in a plasma-chemical reactor based on volume barrier discharge

NASA Astrophysics Data System (ADS)

Soloshenko, I. A.; Tsiolko, V. V.; Pogulay, S. S.; Terent'yeva, A. G.; Bazhenov, V. Yu; Shchedrin, A. I.; Ryabtsev, A. V.; Kuzmichev, A. I.

2007-02-01

In this paper the results of theoretical and experimental studies of the component content of active particles formed in a plasma-chemical reactor composed of a multiple-cell generator of active particles, based on volume barrier discharge, and a working chamber are presented. For calculation of the content of uncharged plasma components an approach is proposed which is based on averaging of the power introduced over the entire volume. Advantages of such an approach lie in an absence of fitting parameters, such as the dimensions of microdischarges, their surface density and rate of breakdown. The calculation and the experiment were accomplished with the use of dry air (20% relative humidity) as the plasma generating medium. Concentrations of O3, HNO3, HNO2, N2 O5 and NO3 were measured experimentally in the discharge volume and working chamber for the residence time of particles on a discharge of 0.3 s and more and discharge specific power of 1.5 W cm-3. It has been determined that the best agreement between the calculation and the experiment occurs at calculated gas medium temperatures in the discharge plasma of about 400-425 K, which correspond to the experimentally measured rotational temperature of nitrogen. In most cases the calculated concentrations of O3, HNO3, HNO2, N2O5 and NO3 for the barrier discharge and the working chamber are in fairly good agreement with the respective measured values.

Decomposition of L-valine under nonthermal dielectric barrier discharge plasma.

PubMed

Li, Yingying; Kojtari, Arben; Friedman, Gary; Brooks, Ari D; Fridman, Alex; Ji, Hai-Feng

2014-02-13

L-Valine solutions in water and phosphate buffer were treated with nonthermal plasma generated by using a dielectric barrier discharge (DBD) device and the products generated after plasma treatments were characterized by (1)H NMR and GC-MS. Our results demonstrate that L-valine is decomposed to acetone, formic acid, acetic acid, threo-methylaspartic acid, erythro-methlyaspartic acid, and pyruvic acid after direct exposure to DBD plasma. The concentrations of these compounds are time-dependent with plasma treatment. The mechanisms of L-valine under the DBD plasma are also proposed in this study. Acetone, pyruvic acid, and organic radicals (•)CHO, CH3COCH2OO(•) (acetonylperoxy), and CH3COC(OH)2OO(•) (1,1-dihydroxypropan-2-one peroxy) may be the determining chemicals in DNA damage.

Application of microplasma discharge in a spark gap for high repetitive switching

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rahaman, Hasibur; Nam, Sang Hoon; Nam, Jong Woo

2010-04-05

The electrical breakdown in a spark gap for repetitive switching has been a long research interest. For this purpose, microplasma discharge is implemented in the spark gap which is further integrated inside a coaxial transmission line. This work addresses important physical properties and insights of the microplasma discharge, to be optimized, such as plasma generation in a spark channel, dielectric recovery process, and residual plasma in the postspark discharge period. Although understanding the microplasma discharge is the primary goal, considerable attention has been focused on an external circuit scheme to drive the discharge system at a high repetition rate.

Numerical simulations of dielectric barrier discharges

NASA Astrophysics Data System (ADS)

Martens, Tom

A plasma or gas discharge is a state of matter which can be described as a gas containing ionized atoms and molecules. This ionized gas exhibits a collective behaviour under influence of an electric or a magnetic field, which are responsible for unique properties which make all new kinds of technology possible. The most important motivation behind the research is finding more efficient ways to produce a low-temperature plasma. In order to achieve this different reactor geometries are studied, it is investigated which is the most suitable power source and the influence of small contaminations of the operating gas is assessed. The studied plasmas are mainly operated at atmospheric pressure. Working at this pressure is cheaper and it makes it possible to develop assembly line treatments. Such plasmas are most easily generated in very small geometries, although energetic derailment of the discharge becomes a substantial risk. This is avoided when the electrodes are electrically insulated. In such setup the insulators accumulate charges which compensate the governing electric field, which keeps the energy transfer to the discharge limited. By studying these discharges using computer models, the changes in the plasma chemistry in time and also under the influence of different levels of impurities were characterized in great detail. Moreover, it was also determined how these chemical changes determine the electrical characteristics of the plasma. Finally, the insights in the charging and discharging effects of the insulators were used to make predictions on which type of power source is the most efficient in using the potential energy stored on the insulator surface to generate the plasma. The most important conclusions are that molecular impurities of the order of only one part per million already dominate the ionic particle distributions in the plasma and that a well-designed alteration in the applied voltage profile leads to a plasma generation with a more than three times more efficient use of consumed energy. This way the research contributes to the insight in the operation and forms the base for new and improved applications and technologies.

Water Treatment Using Plasma Discharge with Variation of Electrode Materials

NASA Astrophysics Data System (ADS)

Chanan, N.; Kusumandari; Saraswati, T. E.

2018-03-01

This research studied water treatment using plasma discharge. Plasma generated in this study produced active species that played a role in organic compound decomposition. The plasma reactor consisted of two needle electrodes made from stainless steel, tungsten, aluminium and grafit. It placed approximately 2 mm above the solution and connected with high-AC voltage. A solution of methylene blue used as an organic solution model. Plasma treatment times were 2, 4, 6, 8 and 10 min. The absorbance, temperature and pH of the solution were measured before and after treatment using various electrodes. The best electrode used in plasma discharging for methylene blue absorbance reduction was the graphite electrode, which provided the highest degradation efficiency of 98% at 6 min of treatment time.

Boundary Layer Flow Control with a One Atmosphere Uniform Glow Discharge Surface Plasma

NASA Technical Reports Server (NTRS)

Roth, J. Reece; Sherman, Daniel M.; Wilkinson, Stephen P.

1998-01-01

Low speed wind tunnel data have been acquired for planar panels covered by a uniform, glow-discharge surface plasma in atmospheric pressure air known as the One Atmosphere Uniform Glow Discharge Plasma (OAUGDP). Streamwise and spanwise arrays of flush, plasma-generating surface electrodes have been studied in laminar, transitional, and fully turbulent boundary layer flow. Plasma between symmetric streamwise electrode strips caused large increases in panel drag, whereas asymmetric spanwise electrode configurations produced a significant thrust. Smoke wire flow visualization and mean velocity diagnostics show the primary cause of the phenomena to be a combination of mass transport and vortical structures induced by strong paraelectric ElectroHydroDynamic (EHD) body forces on the flow.

Solid expellant plasma generator

NASA Technical Reports Server (NTRS)

Stone, Nobie H. (Inventor); Poe, Garrett D. (Inventor); Rood, Robert (Inventor)

2010-01-01

An improved solid expellant plasma generator has been developed. The plasma generator includes a support housing, an electrode rod located in the central portion of the housing, and a mass of solid expellant material that surrounds the electrode rod within the support housing. The electrode rod and the solid expellant material are made of separate materials that are selected so that the electrode and the solid expellant material decompose at the same rate when the plasma generator is ignited. This maintains a point of discharge of the plasma at the interface between the electrode and the solid expellant material.

Controlled cytotoxicity of plasma treated water formulated by open-air hybrid mode discharge

NASA Astrophysics Data System (ADS)

Lu, P.; Boehm, D.; Cullen, P.; Bourke, P.

2017-06-01

Plasma treated liquids (PTLs) provide a means to convey a broad range of effects of relevance for food, environmental, or clinical decontamination, plant growth promotion, and therapeutic applications. Devising the reactive species ingredients and controlling the biological response of PTLs are of great interest. We demonstrate an approach by using an open-air hybrid mode discharge (HMD) to control the principal reactive species composition within plasma treated water (PTW), which is then demonstrated to regulate the cytotoxicity of PTW. The cytotoxicity of HMD produced PTW demonstrates a non-monotonic change over the discharge time. Although hydrogen peroxide and nitrite are not the sole effectors for cell death caused by PTW, using them as principal reactive species indicators, cytotoxicity can be removed and/or enhanced by formulating their concentrations and composition through adjusting the discharge mode and time on-line during PTW generation without the addition of additional working gas or chemical scavengers. This work demonstrates that a hybrid mode discharge can be employed to generate a PTW formulation to control a biological response such as cytotoxicity. This provides insights into how plasma treated liquids may be harnessed for biological applications in a specific and controllable manner.

Characteristics of cold atmospheric plasma source based on low-current pulsed discharge with coaxial electrodes

NASA Astrophysics Data System (ADS)

Bureyev, O. A.; Surkov, Yu S.; Spirina, A. V.

2017-05-01

This work investigates the characteristics of the gas discharge system used to create an atmospheric pressure plasma flow. The plasma jet design with a cylindrical graphite cathode and an anode rod located on the axis of the system allows to realize regularly reproducible spark breakdowns mode with a frequency ∼ 5 kHz and a duration ∼ 40 μs. The device generates a cold atmospheric plasma flame with 1 cm in diameter in the flow of various plasma forming gases including nitrogen and air at about 100 mA average discharge current. In the described construction the cathode spots of individual spark channels randomly move along the inner surface of the graphite electrode creating the secondary plasma stream time-average distributed throughout the whole exit aperture area after the decay of numerous filamentary discharge channels. The results of the spectral diagnostics of plasma in the discharge gap and in the stream coming out of the source are presented. Despite the low temperature of atoms and molecules in plasma stream the cathode spots operation with temperature of ∼ 4000 °C at a graphite electrode inside a discharge system enables to saturate the plasma by CN-radicals and atomic carbon in the case of using nitrogen as the working gas.

Foundations of atmospheric pressure non-equilibrium plasmas

NASA Astrophysics Data System (ADS)

Bruggeman, Peter J.; Iza, Felipe; Brandenburg, Ronny

2017-12-01

Non-equilibrium plasmas have been intensively studied over the past century in the context of material processing, environmental remediation, ozone generation, excimer lamps and plasma display panels. Research on atmospheric pressure non-equilibrium plasmas intensified over the last two decades leading to a large variety of plasma sources that have been developed for an extended application range including chemical conversion, medicine, chemical analysis and disinfection. The fundamental understanding of these discharges is emerging but there remain a lot of unexplained phenomena in these intrinsically complex plasmas. The properties of non-equilibrium plasmas at atmospheric pressure span over a huge range of electron densities as well as heavy particle and electron temperatures. This paper provides an overview of the key underlying processes that are important for the generation and stabilization of atmospheric pressure non-equilibrium plasmas. The unique physical and chemical properties of theses discharges are also summarized.

Method for generating a highly reactive plasma for exhaust gas aftertreatment and enhanced catalyst reactivity

DOEpatents

Whealton, John H.; Hanson, Gregory R.; Storey, John M.; Raridon, Richard J.; Armfield, Jeffrey S.; Bigelow, Timothy S.; Graves, Ronald L.

2002-01-01

A method for non-thermal plasma aftertreatment of exhaust gases the method comprising the steps of providing short risetime, high frequency, high power bursts of low-duty factor microwaves sufficient to generate a plasma discharge and passing a gas to be treated through the discharge so as to cause dissociative reduction of the exhaust gases and enhanced catalyst reactivity through application of the pulsed microwave fields directly to the catalyst material sufficient to cause a polarizability catastrophe and enhanced heating of the metal crystallite particles of the catalyst, and in the presence or absence of the plasma. The invention also includes a reactor for aftertreatment of exhaust gases.

An investigation of transient pressures and plasma properties in a pinched plasma column. M.S. Thesis

NASA Technical Reports Server (NTRS)

Stover, E. K.; York, T. M.

1971-01-01

The transient pinched plasma column generated in a linear Z-pinch was studied experimentally and analytically. The plasma column was investigated experimentally with several plasma diagnostics; they were: a rapid response pressure transducer, a magnetic field probe, a voltage probe, and discharge luminosity. Axial pressure profiles on the discharge chamber axis were used to identify three characteristic regions of plasma column behavior: (1) strong axial pressure asymmetry noted early in plasma column lifetime, (2) followed by plasma heating in which there is a rapid rise in static pressure, and (3) a slight decrease static pressure before plasma column breakup. Plasma column lifetime was approximately 5 microseconds. The axial pressure asymmetry was attributed to nonsimultaneous pinching of the imploding current sheet along the discharge chamber axis. The rapid heating could be attributed in part to viscous effects introduced by radial gradients in the axial streaming velocity.

On production and asymmetric focusing of flat electron beams using rectangular capillary discharge plasmas

DOE PAGES

Bagdasarov, G. A.; Bobrova, N. A.; Boldarev, A. S.; ...

2017-12-27

A method for the asymmetric focusing of electron bunches, based on the active plasma lensing technique is proposed. Our method takes advantage of the strong inhomogeneous magnetic field generated inside the capillary discharge plasma to focus the ultrarelativistic electrons. The plasma and magnetic field parameters inside the capillary discharge are described theoretically and modeled with dissipative magnetohydrodynamic computer simulations enabling analysis of the capillaries of rectangle cross-sections. We could use large aspect ratio rectangular capillaries to transport electron beams with high emittance asymmetries, as well as assist in forming spatially flat electron bunches for final focusing before the interaction point.

On production and asymmetric focusing of flat electron beams using rectangular capillary discharge plasmas

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bagdasarov, G. A.; Bobrova, N. A.; Boldarev, A. S.

A method for the asymmetric focusing of electron bunches, based on the active plasma lensing technique is proposed. Our method takes advantage of the strong inhomogeneous magnetic field generated inside the capillary discharge plasma to focus the ultrarelativistic electrons. The plasma and magnetic field parameters inside the capillary discharge are described theoretically and modeled with dissipative magnetohydrodynamic computer simulations enabling analysis of the capillaries of rectangle cross-sections. We could use large aspect ratio rectangular capillaries to transport electron beams with high emittance asymmetries, as well as assist in forming spatially flat electron bunches for final focusing before the interaction point.

On production and asymmetric focusing of flat electron beams using rectangular capillary discharge plasmas

NASA Astrophysics Data System (ADS)

Bagdasarov, G. A.; Bobrova, N. A.; Boldarev, A. S.; Olkhovskaya, O. G.; Sasorov, P. V.; Gasilov, V. A.; Barber, S. K.; Bulanov, S. S.; Gonsalves, A. J.; Schroeder, C. B.; van Tilborg, J.; Esarey, E.; Leemans, W. P.; Levato, T.; Margarone, D.; Korn, G.; Kando, M.; Bulanov, S. V.

2017-12-01

A method for the asymmetric focusing of electron bunches, based on the active plasma lensing technique, is proposed. This method takes advantage of the strong inhomogeneous magnetic field generated inside the capillary discharge plasma to focus on the ultrarelativistic electrons. The plasma and magnetic field parameters inside the capillary discharge are described theoretically and modeled with dissipative magnetohydrodynamic computer simulations enabling analysis of the capillaries of rectangle cross-sections. Large aspect ratio rectangular capillaries might be used to transport electron beams with high emittance asymmetries, as well as assist in forming spatially flat electron bunches for final focusing before the interaction point.

Confluence or independence of microwave plasma bullets in atmospheric argon plasma jet plumes

NASA Astrophysics Data System (ADS)

Li, Ping; Chen, Zhaoquan; Mu, Haibao; Xu, Guimin; Yao, Congwei; Sun, Anbang; Zhou, Yuming; Zhang, Guanjun

2018-03-01

Plasma bullet is the formation and propagation of a guided ionization wave (streamer), normally generated in atmospheric pressure plasma jet (APPJ). In most cases, only an ionization front produces in a dielectric tube. The present study shows that two or three ionization fronts can be generated in a single quartz tube by using a microwave coaxial resonator. The argon APPJ plumes with a maximum length of 170 mm can be driven by continuous microwaves or microwave pulses. When the input power is higher than 90 W, two or three ionization fronts propagate independently at first; thereafter, they confluence to form a central plasma jet plume. On the other hand, the plasma bullets move independently as the lower input power is applied. For pulsed microwave discharges, the discharge images captured by a fast camera show the ionization process in detail. Another interesting finding is that the strongest lightening plasma jet plumes always appear at the shrinking phase. Both the discharge images and electromagnetic simulations suggest that the confluence or independent propagation of plasma bullets is resonantly excited by the local enhanced electric fields, in terms of wave modes of traveling surface plasmon polaritons.

Fast discharge in a spherical cavity

DOE Office of Scientific and Technical Information (OSTI.GOV)

Antsiferov, P. S., E-mail: Ants@isan.troitsk.ru; Dorokhin, L. A.

2014-04-15

The work is devoted to the study of the plasma, created by a fast discharge in a spherical cavity. The discharge was driven by an inductive storage with plasma erosion opening switch (dI/dt ∼10{sup 12} A/s). The plasma was produced in a spherical cavity (alumina, 11 mm diameter). Xe, Ar, and He at the pressure 80 Pa were used as working gases. The time evolution of the spatial structure and of extreme ultraviolet (EUV) spectra of the discharge plasma was studied by means of micro channel plate detector. The discharges with Xe and Ar resulted in the stable appearance of the spherically shapedmore » plasma with the diameter about 1–3 mm. The plasma emission in the EUV region lasts ∼500 ns. The EUV spectrum of Ar discharge at the moment of maximum of the electron temperature T{sub e} contains the lines of Ar X (ionization potential 478.7 eV), that indicates a value of T{sub e} in the range 50–100 eV. The mechanism of plasma appearance can be the cumulation of the convergent spherical shock wave, generated by fast heat deposition and magnetic pressure in working media near the inner surface of the discharge volume.« less

PLASMA GENERATOR

DOEpatents

Foster, J.S. Jr.

1958-03-11

This patent describes apparatus for producing an electricity neutral ionized gas discharge, termed a plasma, substantially free from contamination with neutral gas particles. The plasma generator of the present invention comprises a plasma chamber wherein gas introduced into the chamber is ionized by a radiofrequency source. A magnetic field is used to focus the plasma in line with an exit. This magnetic field cooperates with a differential pressure created across the exit to draw a uniform and uncontaminated plasma from the plasma chamber.

Study on the plasma generation characteristics of an induction-triggered coaxial pulsed plasma thruster

NASA Astrophysics Data System (ADS)

Weisheng, CUI; Wenzheng, LIU; Jia, TIAN; Xiuyang, CHEN

2018-02-01

At present, spark plugs are used to trigger discharge in pulsed plasma thrusters (PPT), which are known to be life-limiting components due to plasma corrosion and carbon deposition. A strong electric field could be formed in a cathode triple junction (CTJ) to achieve a trigger function under vacuum conditions. We propose an induction-triggered electrode structure on the basis of the CTJ trigger principle. The induction-triggered electrode structure could increase the electric field strength of the CTJ without changing the voltage between electrodes, contributing to a reduction in the electrode breakdown voltage. Additionally, it can maintain the plasma generation effect when the breakdown voltage is reduced in the discharge experiments. The induction-triggered electrode structure could ensure an effective trigger when the ablation distance of Teflon increases, and the magnetic field produced by the discharge current could further improve the plasma density and propagation velocity. The induction-triggered coaxial PPT we propose has a simplified trigger structure, and it is an effective attempt to optimize the micro-satellite thruster.

Characterization of a dielectric barrier discharge in contact with liquid and producing a plasma activated water

NASA Astrophysics Data System (ADS)

Neretti, G.; Taglioli, M.; Colonna, G.; Borghi, C. A.

2017-01-01

In this work a low-temperature plasma source for the generation of plasma activated water (PAW) is developed and characterized. The plasma reactor was operated by means of an atmospheric-pressure air dielectric barrier discharge (DBD). The plasma generated is in contact with the water surface and is able to chemically activate the liquid medium. Electrodes were supplied by both sinusoidal and nanosecond-pulsed voltage waveforms. Treatment times were varied from 2 to 12 min to increase the energy dose released to the water by the DBD plasma. The physics of the discharge was studied by means of electrical, spectroscopic and imaging diagnostics. The interaction between the plasma and the liquid was investigated as well. Temperature and composition of the treated water were detected. Images of the discharges showed a filamentary behaviour in the sinusoidal case and a more homogeneous behaviour in the nanosecond-pulsed one. The images and the electrical measurements allowed to evaluate an average electron number density of about 4  ×  1019 and 6  ×  1017 m-3 for the sinusoidal and nanosecond-pulsed discharges respectively. Electron temperatures in the range of 2.1÷2.6 eV were measured by using spectroscopic diagnostics. Rotational temperatures in the range of 318-475 K were estimated by fitting synthetic spectra with the measured ones. Water temperature and pH level did not change significantly after the exposure to the DBD plasma. The production of ozone and hydrogen peroxide within the water was enhanced by increasing the plasma treatment time and the energy dose. Numerical simulations of the nanosecond-pulsed discharge were performed by using a self-consistent coupling of state-to-state kinetics of the air mixture with the Boltzmann equation of free electron kinetics. Temporal evolution of the electron energy distribution function shows departure from the Maxwellian distribution especially during the afterglow phase of the discharge. When limited deviations from Maxwellian distribution were observed, calculated electron temperature is in good agreement with the one measured by means of spectroscopic diagnostics. Computed temporal evolution of the energy delivered to the discharge is comparable with the one obtained from electrical measurements. The electrical discharges supplied by both voltage waveforms produce plasma activated water with negligible thermal effects and pH variations.

Efficient Radio Frequency Inductive Discharges in Near Atmospheric Pressure Using Immittance Conversion Topology

NASA Astrophysics Data System (ADS)

Razzak, M. Abdur; Takamura, Shuichi; Uesugi, Yoshihiko; Ohno, Noriyasu

A radio frequency (rf) inductive discharge in atmospheric pressure range requires high voltage in the initial startup phase and high power during the steady state sustainment phase. It is, therefore, necessary to inject high rf power into the plasma ensuring the maximum use of the power source, especially where the rf power is limited. In order to inject the maximum possible rf power into the plasma with a moderate rf power source of few kilowatts range, we employ the immittance conversion topology by converting a constant voltage source into a constant current source to generate efficient rf discharge by inductively coupled plasma (ICP) technique at a gas pressure with up to one atmosphere in argon. A novel T-LCL immittance circuit is designed for constant-current high-power operation, which is practically very important in the high-frequency range, to provide high effective rf power to the plasma. The immittance conversion system combines the static induction transistor (SIT)-based radio frequency (rf) high-power inverter circuit and the immittance conversion elements including the rf induction coil. The basic properties of the immittance circuit are studied by numerical analysis and verified the results by experimental measurements with the inductive plasma as a load at a relatively high rf power of about 4 kW. The performances of the immittance circuit are also evaluated and compared with that of the conventional series resonance circuit in high-pressure induction plasma generation. The experimental results reveal that the immittance conversion circuit confirms injecting higher effective rf power into the plasma as much as three times than that of the series resonance circuit under the same operating conditions and same dc supply voltage to the inverter, thereby enhancing the plasma heating efficiency to generate efficient rf inductive discharges.

Electrical method for the measurements of volume averaged electron density and effective coupled power to the plasma bulk

NASA Astrophysics Data System (ADS)

Henault, M.; Wattieaux, G.; Lecas, T.; Renouard, J. P.; Boufendi, L.

2016-02-01

Nanoparticles growing or injected in a low pressure cold plasma generated by a radiofrequency capacitively coupled capacitive discharge induce strong modifications in the electrical parameters of both plasma and discharge. In this paper, a non-intrusive method, based on the measurement of the plasma impedance, is used to determine the volume averaged electron density and effective coupled power to the plasma bulk. Good agreements are found when the results are compared to those given by other well-known and established methods.

Electron density measurement in gas discharge plasmas by optical and acoustic methods

NASA Astrophysics Data System (ADS)

Biagioni, A.; Anania, M. P.; Bellaveglia, M.; Chiadroni, E.; Cianchi, A.; Di Giovenale, D.; Di Pirro, G.; Ferrario, M.; Filippi, F.; Mostacci, A.; Pompili, R.; Shpakov, V.; Vaccarezza, C.; Villa, F.; Zigler, A.

2016-08-01

Plasma density represents a very important parameter for both laser wakefield and plasma wakefield acceleration, which use a gas-filled capillary plasma source. Several techniques can be used to measure the plasma density within a capillary discharge, which are mainly based on optical diagnostic methods, as for example the well-known spectroscopic method using the Stark broadening effect. In this work, we introduce a preliminary study on an alternative way to detect the plasma density, based on the shock waves produced by gas discharge in a capillary. Firstly, the measurements of the acoustic spectral content relative to the laser-induced plasmas by a solid target allowed us to understand the main properties of the acoustic waves produced during this kind of plasma generation; afterwards, we have extended such acoustic technique to the capillary plasma source in order to calibrate it by comparison with the stark broadening method.

Plasma sterilization of polyethylene terephthalate bottles by pulsed corona discharge at atmospheric pressure.

PubMed

Masaoka, Satoshi

2007-06-01

A pulsed power supply was used to generate a corona discharge on a polyethylene terephthalate bottle, to conduct plasma sterilization at atmospheric pressure. Before generating such a discharge, minute quantities of water were attached to the inner surface of the bottle and to the surface of a high voltage (HV) electrode inserted into the bottle. Next, high-voltage pulses of electricity were discharged between electrodes for 6.0s, while rotating the bottle. The resulting spore log reduction values of Bacillus subtilis and Aspergillus niger on the inner surface of the bottle were 5.5 and 6 or higher, respectively, and those on the HV electrode surface were each 6 or higher for both strains. The presence of the by-products gaseous ozone, hydrogen peroxide, and nitric ions resulting from the electrical discharge was confirmed.

Sterilization of Turmeric by Atmospheric Pressure Dielectric Barrier Discharge Plasma

NASA Astrophysics Data System (ADS)

Setareh, Salarieh; Davoud, Dorranian

2013-11-01

In this study atmospheric pressure dielectric barrier discharge (DBD) plasma has been employed for sterilizing dry turmeric powders. A 6 kV, 6 kHz frequency generator was used to generate plasma with Ar, Ar/O2, He, and He/O2 gases between the 5 mm gap of two quartz covered electrodes. The complete sterilization time of samples due to plasma treatment was measured. The most important contaminant of turmeric is bacillus subtilis. The results show that the shortest sterilization time of 15 min is achieved by exposing the samples to Ar/O2 plasma. Survival curves of samples are exponential functions of time and the addition of oxygen to plasma leads to a significant increase of the absolute value of time constant of the curves. Magnitudes of protein and DNA in treated samples were increased to a similar value for all samples. Taste, color, and solubility of samples were not changed after the plasma treatment.

Inactivation of possible micromycete food contaminants using the low-temperature plasma and hydrogen peroxide

NASA Astrophysics Data System (ADS)

Čeřovský, M.; Khun, J.; Rusová, K.; Scholtz, V.; Soušková, H.

2013-09-01

The inhibition effect of hydrogen peroxide aerosol, low-temperature plasma and their combinations has been studied on several micromycetes spores. The low-temperature plasma was generated in corona discharges in the open air apparatus with hydrogen peroxide aerosol. Micromycete spores were inoculated on the surface of agar plates, exposed solely to the hydrogen peroxide aerosol, corona discharge or their combination. After incubation the diameter of inhibition zone was measured. The solely positive corona discharge exhibits no inactivation effect, the solely negative corona discharge and solely hydrogen peroxide aerosol exhibit the inactivation effect, however their combinations exhibit to be much more effective. Low-temperature plasma and hydrogen peroxide aerosol present a possible alternative method of microbial decontamination of food, food packages or other thermolabile materials.

Inactivation of possible micromycete food contaminants using the low-temperature plasma and hydrogen peroxide

DOE Office of Scientific and Technical Information (OSTI.GOV)

Čeřovský, M., E-mail: scholtz@aldebaran.cz; Khun, J.; Rusová, K.

2013-09-15

The inhibition effect of hydrogen peroxide aerosol, low-temperature plasma and their combinations has been studied on several micromycetes spores. The low-temperature plasma was generated in corona discharges in the open air apparatus with hydrogen peroxide aerosol. Micromycete spores were inoculated on the surface of agar plates, exposed solely to the hydrogen peroxide aerosol, corona discharge or their combination. After incubation the diameter of inhibition zone was measured. The solely positive corona discharge exhibits no inactivation effect, the solely negative corona discharge and solely hydrogen peroxide aerosol exhibit the inactivation effect, however their combinations exhibit to be much more effective. Low-temperaturemore » plasma and hydrogen peroxide aerosol present a possible alternative method of microbial decontamination of food, food packages or other thermolabile materials.« less

Post-breakdown secondary discharges at the electrode/dielectric interface of a cylindrical barrier discharge

NASA Astrophysics Data System (ADS)

Carman, Robert; Ward, Barry; Kane, Deborah

2011-10-01

The electrical breakdown characteristics of a double-walled cylindrical dielectric barrier discharge (DBD) lamp with a neon buffer gas under pulsed voltage excitation have been investigated. Following the formation of plasma in the main discharge gap, we have observed secondary breakdown phenomena at the inner and outer mesh electrode/dielectric interfaces under specific operating conditions. Plasma formation at these interfaces is investigated by monitoring the Ozone production rate in controlled flows of ultra high purity oxygen together with the overall electrical voltage-charge characteristics of the lamp. The results show that this secondary breakdown only occurs after the main discharge plasma has been established, and that significant electrical power may be dissipated in generating these spurious secondary plasmas. The results are important with regards to optimising the design and identifying efficient operating regimes of DBD based devices that employ mesh-type or wire/strip electrodes.

[Study on the Emission Spectrum of Hydrogen Production with Microwave Discharge Plasma in Ethanol Solution].

PubMed

Sun, Bing; Wang, Bo; Zhu, Xiao-mei; Yan, Zhi-yu; Liu, Yong-jun; Liu, Hui

2016-03-01

Hydrogen is regarded as a kind of clean energy with high caloricity and non-pollution, which has been studied by many experts and scholars home and abroad. Microwave discharge plasma shows light future in the area of hydrogen production from ethanol solution, providing a new way to produce hydrogen. In order to further improve the technology and analyze the mechanism of hydrogen production with microwave discharge in liquid, emission spectrum of hydrogen production by microwave discharge plasma in ethanol solution was being studied. In this paper, plasma was generated on the top of electrode by 2.45 GHz microwave, and the spectral characteristics of hydrogen production from ethanol by microwave discharge in liquid were being studied using emission spectrometer. The results showed that a large number of H, O, OH, CH, C2 and other active particles could be produced in the process of hydrogen production from ethanol by microwave discharge in liquid. The emission spectrum intensity of OH, H, O radicals generated from ethanol is far more than that generated from pure water. Bond of O-H split by more high-energy particles from water molecule was more difficult than that from ethanol molecule, so in the process of hydrogen production by microwave discharge plasma in ethanol solution; the main source of hydrogen was the dehydrogenation and restructuring of ethanol molecules instead of water decomposition. Under the definite external pressure and temperature, the emission spectrum intensity of OH, H, O radicals increased with the increase of microwave power markedly, but the emission spectrum intensity of CH, C2 active particles had the tendency to decrease with the increase of microwave power. It indicated that the number of high energy electrons and active particles high energy electron energy increased as the increase of microwave power, so more CH, C2 active particles were split more thoroughly.

Ozone generation in a kHz-pulsed He-O2 capillary dielectric barrier discharge operated in ambient air

NASA Astrophysics Data System (ADS)

Sands, Brian L.; Ganguly, Biswa N.

2013-12-01

The generation of reactive oxygen species using nonequilibrium atmospheric pressure plasma jet devices has been a subject of recent interest due to their ability to generate localized concentrations from a compact source. To date, such studies with plasma jet devices have primarily utilized radio-frequency excitation. In this work, we characterize ozone generation in a kHz-pulsed capillary dielectric barrier discharge configuration comprised of an active discharge plasma jet operating in ambient air that is externally grounded. The plasma jet flow gas was composed of helium with an admixture of up to 5% oxygen. A unipolar voltage pulse train with a 20 ns pulse risetime was used to drive the discharge at repetition rates between 2-25 kHz. Using UVLED absorption spectroscopy centered at 255 nm near the Hartley-band absorption peak, ozone was detected over 1 cm from the capillary axis. We observed roughly linear scaling of ozone production with increasing pulse repetition rate up to a "turnover frequency," beyond which ozone production steadily dropped and discharge current and 777 nm O(5P→5S°) emission sharply increased. The turnover in ozone production occurred at higher pulse frequencies with increasing flow rate and decreasing applied voltage with a common energy density of 55 mJ/cm3 supplied to the discharge. The limiting energy density and peak ozone production both increased with increasing O2 admixture. The power dissipated in the discharge was obtained from circuit current and voltage measurements using a modified parallel plate dielectric barrier discharge circuit model and the volume-averaged ozone concentration was derived from a 2D ozone absorption measurement. From these measurements, the volume-averaged efficiency of ozone production was calculated to be 23 g/kWh at conditions for peak ozone production of 41 mg/h at 11 kV applied voltage, 3% O2, 2 l/min flow rate, and 13 kHz pulse repetition rate, with 1.79 W dissipated in the discharge.

A compact, low cost Marx bank for generating capillary discharge plasmas.

PubMed

Dyson, A E; Thornton, C; Hooker, S M

2016-09-01

We describe in detail a low power Compact Marx Bank (CMB) circuit that can provide 20 kV, 500 A pulses of approximately 100-200 ns duration. One application is the generation of capillary discharge plasmas of density ≈10 18 cm -3 used in laser plasma accelerators. The CMB is triggered with a high speed solid state switch and gives a high voltage output pulse with a ns scale rise time into a 50 Ω load (coaxial cable) with <4 ns voltage jitter. Its small size (10 cm  ×  25 cm  ×  5 cm) means that it can be placed right next to the capillary discharge in the target chamber to avoid the need to impedance match. The electrical energy required per discharge is <1 J, and the CMB can be run at shot repetition rates of ≳1 Hz. This low power requirement means that the circuit can easily be powered by a small lead acid battery and, therefore, can be floated relative to laboratory earth. The CMB is readily scalable and pulses >45 kV are demonstrated in air discharges.

A compact, low cost Marx bank for generating capillary discharge plasmas

NASA Astrophysics Data System (ADS)

Dyson, A. E.; Thornton, C.; Hooker, S. M.

2016-09-01

We describe in detail a low power Compact Marx Bank (CMB) circuit that can provide 20 kV, 500 A pulses of approximately 100-200 ns duration. One application is the generation of capillary discharge plasmas of density ≈1018 cm-3 used in laser plasma accelerators. The CMB is triggered with a high speed solid state switch and gives a high voltage output pulse with a ns scale rise time into a 50 Ω load (coaxial cable) with <4 ns voltage jitter. Its small size (10 cm × 25 cm × 5 cm) means that it can be placed right next to the capillary discharge in the target chamber to avoid the need to impedance match. The electrical energy required per discharge is <1 J, and the CMB can be run at shot repetition rates of ≳1 Hz. This low power requirement means that the circuit can easily be powered by a small lead acid battery and, therefore, can be floated relative to laboratory earth. The CMB is readily scalable and pulses >45 kV are demonstrated in air discharges.

Alfvén oscillations in ohmic discharges with runaway electrons in the TUMAN-3M tokamak

NASA Astrophysics Data System (ADS)

Tukachinsky, A. S.; Askinazi, L. G.; Balachenkov, I. M.; Belokurov, A. A.; Gin, D. B.; Zhubr, N. A.; Kornev, V. A.; Lebedev, S. V.; Khil'kevich, E. M.; Chugunov, I. N.; Shevelev, A. E.

2016-12-01

Studying the mechanism of Alfvén wave generation in plasma is important, since the interaction of these waves with energetic particles in tokamak-type reactors can increase the losses of energy and particles with the corresponding decrease in the efficiency of plasma heating and, under certain conditions, lead to the damage of structural elements of the system. Despite the previous detailed investigations of the excitation of Alfvén waves by superthermal particles in regimes with additional heating, the physics of Alfvén mode generation in discharges with ohmic heating of plasma is still not sufficiently studied. We have established that a significant factor inf luencing the development of Alfvén oscillations in ohmic discharge is the presence of runaway electrons. A physical mechanism explaining this relationship is proposed.

Development of soft ionization using direct current pulse glow discharge plasma source in mass spectrometry for volatile organic compounds analysis

NASA Astrophysics Data System (ADS)

Nunome, Yoko; Kodama, Kenji; Ueki, Yasuaki; Yoshiie, Ryo; Naruse, Ichiro; Wagatsuma, Kazuaki

2018-01-01

This study describes an ionization source for mass analysis, consisting of glow discharge plasma driven by a pulsed direct-current voltage for soft plasma ionization, to detect toxic volatile organic compounds (VOCs) rapidly and easily. The novelty of this work is that a molecular adduct ion, in which the parent molecule attaches with an NO+ radical, [M + NO]+, can be dominantly detected as a base peak with little or no fragmentation of them in an ambient air plasma at a pressure of several kPa. Use of ambient air as the discharge plasma gas is suitable for practical applications. The higher pressure in an ambient air discharge provided a stable glow discharge plasma, contributing to the soft ionization of organic molecules. Typical mass spectra of VOCs toluene, benzene, o-xylene, chlorobenzene and n-hexane were observed as [M + NO]+ adduct ion whose peaks were detected at m/z 122, 108, 136, 142 and 116, respectively. The NO generation was also confirmed by emission bands of NO γ-system. The ionization reactions were suggested, such that NO+ radical formed in an ambient air discharge could attach with the analyte molecule.

Plasma Perturbations in High-Speed Probing of Hall Thruster Discharge Chambers: Quantification and Mitigation

NASA Technical Reports Server (NTRS)

Jorns, Benjamin A.; Goebel, Dan M.; Hofer, Richard R.

2015-01-01

An experimental investigation is presented to quantify the effect of high-speed probing on the plasma parameters inside the discharge chamber of a 6-kW Hall thruster. Understanding the nature of these perturbations is of significant interest given the importance of accurate plasma measurements for characterizing thruster operation. An array of diagnostics including a high-speed camera and embedded wall probes is employed to examine in real time the changes in electron temperature and plasma potential induced by inserting a high-speed reciprocating Langmuir probe into the discharge chamber. It is found that the perturbations onset when the scanning probe is downstream of the electron temperature peak, and that along channel centerline, the perturbations are best characterized as a downstream shift of plasma parameters by 15-20% the length of the discharge chamber. A parametric study is performed to investigate techniques to mitigate the observed probe perturbations including varying probe speed, probe location, and operating conditions. It is found that the perturbations largely disappear when the thruster is operated at low power and low discharge voltage. The results of this mitigation study are discussed in the context of recommended methods for generating unperturbed measurements of the discharge chamber plasma.

Interplay between discharge physics, gas phase chemistry and surface processes in hydrocarbon plasmas

NASA Astrophysics Data System (ADS)

Hassouni, Khaled

2013-09-01

In this paper we present two examples that illustrate two different contexts of the interplay between plasma-surface interaction process and discharge physics and gas phase chemistry in hydrocarbon discharges. In the first example we address the case of diamond deposition processes and illustrate how a detailed investigation of the discharge physics, collisional processes and transport phenomena in the plasma phase make possible to accurately predict the key local-parameters, i.e., species density at the growing substrate, as function of the macroscopic process parameters, thus allowing for a precise control of diamond deposition process. In the second example, we illustrate how the interaction between a rare gas pristine discharge and carbon (graphite) electrode induce a dramatic change on the discharge nature, i.e., composition, ionization kinetics, charge equilibrium, etc., through molecular growth and clustering processes, solid particle formation and dusty plasma generation. Work done in collaboration with Alix Gicquel, Francois Silva, Armelle Michau, Guillaume Lombardi, Xavier Bonnin, Xavier Duten, CNRS, Universite Paris 13.

Catalytic Reactor For Oxidizing Mercury Vapor

DOEpatents

Helfritch, Dennis J.

1998-07-28

A catalytic reactor (10) for oxidizing elemental mercury contained in flue gas is provided. The catalyst reactor (10) comprises within a flue gas conduit a perforated corona discharge plate (30a, b) having a plurality of through openings (33) and a plurality of projecting corona discharge electrodes (31); a perforated electrode plate (40a, b, c) having a plurality of through openings (43) axially aligned with the through openings (33) of the perforated corona discharge plate (30a, b) displaced from and opposing the tips of the corona discharge electrodes (31); and a catalyst member (60a, b, c, d) overlaying that face of the perforated electrode plate (40a, b, c) opposing the tips of the corona discharge electrodes (31). A uniformly distributed corona discharge plasma (1000) is intermittently generated between the plurality of corona discharge electrode tips (31) and the catalyst member (60a, b, c, d) when a stream of flue gas is passed through the conduit. During those periods when corona discharge (1000) is not being generated, the catalyst molecules of the catalyst member (60a, b, c, d) adsorb mercury vapor contained in the passing flue gas. During those periods when corona discharge (1000) is being generated, ions and active radicals contained in the generated corona discharge plasma (1000) desorb the mercury from the catalyst molecules of the catalyst member (60a, b, c, d), oxidizing the mercury in virtually simultaneous manner. The desorption process regenerates and activates the catalyst member molecules.

Parallel 3-D numerical simulation of dielectric barrier discharge plasma actuators

NASA Astrophysics Data System (ADS)

Houba, Tomas

Dielectric barrier discharge plasma actuators have shown promise in a range of applications including flow control, sterilization and ozone generation. Developing numerical models of plasma actuators is of great importance, because a high-fidelity parallel numerical model allows new design configurations to be tested rapidly. Additionally, it provides a better understanding of the plasma actuator physics which is useful for further innovation. The physics of plasma actuators is studied numerically. A loosely coupled approach is utilized for the coupling of the plasma to the neutral fluid. The state of the art in numerical plasma modeling is advanced by the development of a parallel, three-dimensional, first-principles model with detailed air chemistry. The model incorporates 7 charged species and 18 reactions, along with a solution of the electron energy equation. To the author's knowledge, a parallel three-dimensional model of a gas discharge with a detailed air chemistry model and the solution of electron energy is unique. Three representative geometries are studied using the gas discharge model. The discharge of gas between two parallel electrodes is used to validate the air chemistry model developed for the gas discharge code. The gas discharge model is then applied to the discharge produced by placing a dc powered wire and grounded plate electrodes in a channel. Finally, a three-dimensional simulation of gas discharge produced by electrodes placed inside a riblet is carried out. The body force calculated with the gas discharge model is loosely coupled with a fluid model to predict the induced flow inside the riblet.

Post-discharge gas composition of a large-gap DBD in humid air by UV-Vis absorption spectroscopy

NASA Astrophysics Data System (ADS)

Moiseev, T.; Misra, N. N.; Patil, S.; Cullen, P. J.; Bourke, P.; Keener, K. M.; Mosnier, J. P.

2014-12-01

Large gap dielectric barrier discharges (DBD) provide non-thermal, non-equilibrium plasmas that can generate specific gas chemistry with enhanced bactericidal effects when working in humid air. The present study investigates the post-discharge gas composition of such plasmas operated in humid air using UV-Vis (200-800 nm) absorption spectroscopy. Absorbance spectra have been de-convoluted using direct deconvolution and iterative methods and results are correlated to the DBD electrical parameters. The high-voltage (56 and 70 kV rms) DBD plasma generated at 50 Hz frequency in a closed container over a 20 mm gap in air with relative humidity (RH) of 5-70% has been characterized by I-V and capacitive methods. The post-discharge gas composition at each RH is assessed by UV-Vis absorption spectroscopy for plasma exposure times of 15-120 s. The concentration of ozone and nitrogen oxides (O3, NO2, NO3, N2O4) increases with plasma exposure time but a strong decrease in [O3] levels is obtained with increase in RH. The decrease in [O3] and an abundance of nitrogen oxides is ascribed to high specific power densities in the closed container and to increasing RH levels. The absorbance residual following deconvolution shows a strong band at 230-270 nm consistent with the presence of pernitric acid (HNO4) and other HNOx (x = 1, 3) species. Humid air large gap DBD plasmas in closed containers generate along with O3, high levels of nitrogen oxides and HNOx (x = 1, 4) acids leading to increased bactericidal rates.

Analysis and characterization of microwave plasma generated with rectangular all-dielectric resonators

NASA Astrophysics Data System (ADS)

Kourtzanidis, K.; Raja, L. L.

2017-04-01

We report on a computational modeling study of small scale plasma discharge formation with rectangular dielectric resonators (DR). An array of rectangular dielectric slabs, separated by a gap of millimeter dimensions is used to provide resonant response when illuminated by an incident wave of 1.26 GHz. A coupled electromagnetic (EM) wave-plasma model is used to describe the breakdown, early response and steady state of the argon discharge. We characterize the plasma generation with respect to the input power, background gas pressure and gap size. It is found that the plasma discharge is generated mainly inside the gaps between the DR at positions that correspond to the antinodes of the resonant enhanced electric field pattern. The enhancement of the electric field inside the gaps is due to a combination of leaking and displacement current radiation from the DR. The plasma is sustained in over-critical densities due to the large skin depth with respect to the gap and plasma size. Electron densities are calculated in the order of {10}18{--}{10}19 {{{m}}}-3 for a gas pressure of 10 Torr, while they exceed 1020 {{{m}}}-3 in atmospheric conditions. Increase of input power leads to more intense ionization and thus faster plasma formation and results to a more symmetric plasma pattern. For low background gas pressure the discharge is diffusive and extends away from the gap region while in high pressure it is constricted inside the gap. An optimal gap size can be found to provide maximum EM energy transfer to the plasma. This fact demonstrates that the gap size dictates to a certain extent the resonant frequency and the Q-factor of the dielectric array and the breakdown fields can not be determined in a straight-forward way but they are functions of the resonators geometry and incident field frequency.

Experimental characterization of plasma formation and shockwave propagation induced by high power pulsed underwater electrical discharge.

PubMed

Claverie, A; Deroy, J; Boustie, M; Avrillaud, G; Chuvatin, A; Mazanchenko, E; Demol, G; Dramane, B

2014-06-01

High power pulsed electrical discharges into liquids are investigated for new industrial applications based on the efficiency of controlled shock waves. We present here new experimental data obtained by combination of detailed high speed imaging equipments. It allows the visualization of the very first instants of plasma discharge formation, and then the pulsations of the gaseous bubble with an accurate timing of events. The time history of the expansion/compression of this bubble leads to an estimation of the energy effectively transferred to water during the discharge. Finally, the consecutive shock generation driven by this pulsating bubble is optically monitored by shadowgraphs and schlieren setup. These data provide essential information about the geometrical pattern and chronometry associated with the shock wave generation and propagation.

Apparatus for generating quasi-free-space microwave-driven plasmas

NASA Astrophysics Data System (ADS)

Hoff, Brad W.; French, David M.; Reid, Remington R.; Lawrance, Julie E.; Lepell, P. David; Maestas, Sabrina S.

2016-03-01

An apparatus for generating quasi-free-space microwave-driven plasmas has been designed, constructed, and tested. The plasma is driven by a multi-kW, ˜5 GHz microwave beam focused at the center of a vacuum chamber using a Koch-type metal plate lens. Sustained plasma discharges have been generated in argon at pressures ranging from 150 to 200 mTorr, at beam power levels ranging from 5 to 10 kW, and at gas flow rates of approximately 200 SCCM.

Apparatus for generating quasi-free-space microwave-driven plasmas

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hoff, Brad W.; French, David M.; Reid, Remington R.

An apparatus for generating quasi-free-space microwave-driven plasmas has been designed, constructed, and tested. The plasma is driven by a multi-kW, ∼5 GHz microwave beam focused at the center of a vacuum chamber using a Koch-type metal plate lens. Sustained plasma discharges have been generated in argon at pressures ranging from 150 to 200 mTorr, at beam power levels ranging from 5 to 10 kW, and at gas flow rates of approximately 200 SCCM.

Apparatus for generating quasi-free-space microwave-driven plasmas.

PubMed

Hoff, Brad W; French, David M; Reid, Remington R; Lawrance, Julie E; Lepell, P David; Maestas, Sabrina S

2016-03-01

An apparatus for generating quasi-free-space microwave-driven plasmas has been designed, constructed, and tested. The plasma is driven by a multi-kW, ∼5 GHz microwave beam focused at the center of a vacuum chamber using a Koch-type metal plate lens. Sustained plasma discharges have been generated in argon at pressures ranging from 150 to 200 mTorr, at beam power levels ranging from 5 to 10 kW, and at gas flow rates of approximately 200 SCCM.

Method for plasma formation for extreme ultraviolet lithography-theta pinch

DOEpatents

Hassanein, Ahmed [Naperville, IL; Konkashbaev, Isak [Bolingbrook, IL; Rice, Bryan [Hillsboro, OR

2007-02-20

A device and method for generating extremely short-wave ultraviolet electromagnetic wave, utilizing a theta pinch plasma generator to produce electromagnetic radiation in the range of 10 to 20 nm. The device comprises an axially aligned open-ended pinch chamber defining a plasma zone adapted to contain a plasma generating gas within the plasma zone; a means for generating a magnetic field radially outward of the open-ended pinch chamber to produce a discharge plasma from the plasma generating gas, thereby producing a electromagnetic wave in the extreme ultraviolet range; a collecting means in optical communication with the pinch chamber to collect the electromagnetic radiation; and focusing means in optical communication with the collecting means to concentrate the electromagnetic radiation.

Sterilization by negative and positive DC plasma with a micro discharge gap at atmospheric pressure

NASA Astrophysics Data System (ADS)

Li, Hua; Jiang, Lin-Xiu; Jiang, Yong-Rong; Zhu, Jian-Min; Chen, Zhen-Cheng

2017-11-01

A new needle-to-droplet electrode structure with a micro discharge gap (2 mm) was designed to achieve direct current (DC) discharge plasma in ambient air with the aim of using the plasma to sterilize liquids. Without using noble gases or an external air flow, we succeeded in generating both a negative and positive DC plasma at atmospheric pressure. The plasma was driven by a 0 to -20,000 V, 100 W DC power supply. A stainless steel needle with a tip diameter of ˜ 50μm and a 200-μL droplet of bacteria-containing liquid served as the electrodes. At atmospheric pressure and room temperature (23∘C), utilizing the negative DC plasma, the discharge time lasted 10 s; the results showed that the higher the discharge voltage, the more efficient the sterilization effect. Conversely, when we applied a voltage of -5.5 kV, we found that the sterilization effect was more efficient for longer discharge times. Our findings demonstrate that Escherichia coli (E. coli) and Bacillus subtilis (B. subtilis) can be killed in about 30 s. Our experiments show that our sterilization method required less time and was more efficient for positive than for negative DC plasma under the same conditions.

Repetitively Pulsed Nonequilibrium Plasmas for Plasma-Assisted Combustion, Flow Control, and Molecular Lasers

NASA Astrophysics Data System (ADS)

Adamovich, Igor

2006-10-01

The paper presents results of three experiments using high voltage, short pulse duration, high repetition rate discharge plasmas. High electric field during the pulse (E/N˜500-1000 Td) allows efficient ionization and molecular dissociation. Between the pulses, additional energy can be coupled to the decaying plasma using a DC field set below the breakdown threshold. While the DC sustainer discharge adds 90-95% of all the power to the flow, it does not produce any additional ionization. The pulser and the sustainer discharges are fully overlapped in space. Low duty cycle of the pulsed ionizer, ˜1/1000, allows sustaining diffuse and uniform pulser-sustainer plasmas at high pressures and power loadings. The first experiment using the pulsed discharge is ignition of premixed hydrocarbon-air flows, which occurs at low pulsed discharge powers, ˜100 W, and very low plasma temperatures, 100-200^0 C. The second experiment is Lorentz force acceleration of low-temperature supersonic flows. The pulsed discharge was used to generate electrical conductivity in M=3 nitrogen and air flows, while the sustainer discharge produced transverse current in the presence of magnetic field of B=1.5 T. Retarding Lorentz force applied to the flow produced a static pressure increase of up to 15-20%, while accelerating force of the same magnitude resulted in static pressure rise of up to 7-8%, i.e. a factor of two smaller. The third experiment is singlet delta oxygen (SDO) generation in a high-pressure pulser-sustainer discharge. SDO yield was inferred from the integrated intensity of SDO infrared emission spectra calibrated using a blackbody source. The measured yield exceeds the laser threshold yield by about a factor of three, which makes possible achieving positive gain in the laser cavity. The highest gain measured so far is 0.03%/cm.

High density plasma gun generates plasmas at 190 kilometers per second

NASA Technical Reports Server (NTRS)

Espy, P. N.

1971-01-01

Gun has thin metal foil disc which positions or localizes gas to be ionized during electrical discharge cycle, overcoming major limiting factor in obtaining such plasmas. Expanding plasma front travels at 190 km/sec, compared to plasmas of 50 to 60 km/sec previously achieved.

Subnanosecond breakdown in high-pressure gases

NASA Astrophysics Data System (ADS)

Naidis, George V.; Tarasenko, Victor F.; Babaeva, Natalia Yu; Lomaev, Mikhail I.

2018-01-01

Pulsed discharges in high-pressure gases are of considerable interest as sources of nonequilibrium plasma for various technological applications: pollution control, pumping of laser media, plasma-assisted combustion, etc. Recently, attention has been attracted to the use of subnanosecond voltage fronts, producing diffuse discharges with radii of several millimeters. Such plasma structures, similar to pulsed glow discharges, are of special interest for applications due to quasi-uniformity of plasma parameters in relatively large gas volumes. This review presents the results of experimental and computational study of subnanosecond diffuse discharge formation. A description of generators of short high-voltage pulses with subnanosecond fronts and of discharge setups is given. Diagnostic methods for the measurement of various discharge parameters with high temporal and spatial resolution are described. Obtained experimental data on plasma properties for a wide range of governing factors are discussed. A review of various theoretical approaches used for computational study of the dynamics and structure of fast ionization waves is given; the applicability of conventional fluid streamer models for simulation of subnanosecond ionization waves is discussed. Calculated spatial-temporal profiles of plasma parameters during streamer propagation are presented. The efficiency of subnanosecond discharges for the production of reactive species is evaluated. On the basis of the comparison of simulation results and experimental data the effects of various factors (voltage rise time, polarity, etc.) on discharge characteristics are revealed. The major physical phenomena governing the properties of subnanosecond breakdown are analyzed.

Collective Phenomena In Volume And Surface Barrier Discharges

NASA Astrophysics Data System (ADS)

Kogelschatz, U.

2010-07-01

Barrier discharges are increasingly used as a cost-effective means to produce non-equilibrium plasmas at atmospheric pressure. This way, copious amounts of electrons, ions, free radicals and excited species can be generated without appreciable gas heating. In most applications the barrier is made of dielectric material. In laboratory experiments also the use of resistive, ferroelectric and semiconducting materials has been investigated, also porous ceramic layers and dielectric barriers with controlled surface conductivity. Major applications utilizing mainly dielectric barriers include ozone generation, surface cleaning and modification, polymer and textile treatment, sterilization, pollution control, CO2 lasers, excimer lamps, plasma display panels (flat TV screens). More recent research efforts are also devoted to biomedical applications and to plasma actuators for flow control. Sinu- soidal feeding voltages at various frequencies as well as pulsed excitation schemes are used. Volume as well as surface barrier discharges can exist in the form of filamentary, regularly patterned or laterally homogeneous discharges. Reviews of the subject and the older literature on barrier discharges were published by Kogelschatz (2002, 2003), by Wagner et al. (2003) and by Fridman et al. (2005). A detailed discussion of various properties of barrier discharges can also be found in the recent book "Non-Equilibrium Air Plasmas at Atmospheric Pressure" by Becker et al. (2005). The physical effects leading to collective phenomena in volume and surface barrier discharges will be discussed in detail. Special attention will be given to self-organization of current filaments. Main similarities and differences of the two types of barrier discharges will be elaborated.

Development of a plasma generator for a long pulse ion source for neutral beam injectors.

PubMed

Watanabe, K; Dairaku, M; Tobari, H; Kashiwagi, M; Inoue, T; Hanada, M; Jeong, S H; Chang, D H; Kim, T S; Kim, B R; Seo, C S; Jin, J T; Lee, K W; In, S R; Oh, B H; Kim, J; Bae, Y S

2011-06-01

A plasma generator for a long pulse H(+)/D(+) ion source has been developed. The plasma generator was designed to produce 65 A H(+)/D(+) beams at an energy of 120 keV from an ion extraction area of 12 cm in width and 45 cm in length. Configuration of the plasma generator is a multi-cusp bucket type with SmCo permanent magnets. Dimension of a plasma chamber is 25 cm in width, 59 cm in length, and 32.5 cm in depth. The plasma generator was designed and fabricated at Japan Atomic Energy Agency. Source plasma generation and beam extraction tests for hydrogen coupling with an accelerator of the KSTAR ion source have been performed at the KSTAR neutral beam test stand under the agreement of Japan-Korea collaborative experiment. Spatial uniformity of the source plasma at the extraction region was measured using Langmuir probes and ±7% of the deviation from an averaged ion saturation current density was obtained. A long pulse test of the plasma generation up to 200 s with an arc discharge power of 70 kW has been successfully demonstrated. The arc discharge power satisfies the requirement of the beam production for the KSTAR NBI. A 70 keV, 41 A, 5 s hydrogen ion beam has been extracted with a high arc efficiency of 0.9 -1.1 A/kW at a beam extraction experiment. A deuteron yield of 77% was measured even at a low beam current density of 73 mA/cm(2). © 2011 American Institute of Physics

Effect of Dielectric and Liquid on Plasma Sterilization Using Dielectric Barrier Discharge Plasma

PubMed Central

Mastanaiah, Navya; Johnson, Judith A.; Roy, Subrata

2013-01-01

Plasma sterilization offers a faster, less toxic and versatile alternative to conventional sterilization methods. Using a relatively small, low temperature, atmospheric, dielectric barrier discharge surface plasma generator, we achieved ≥6 log reduction in concentration of vegetative bacterial and yeast cells within 4 minutes and ≥6 log reduction of Geobacillus stearothermophilus spores within 20 minutes. Plasma sterilization is influenced by a wide variety of factors. Two factors studied in this particular paper are the effect of using different dielectric substrates and the significance of the amount of liquid on the dielectric surface. Of the two dielectric substrates tested (FR4 and semi-ceramic (SC)), it is noted that the FR4 is more efficient in terms of time taken for complete inactivation. FR4 is more efficient at generating plasma as shown by the intensity of spectral peaks, amount of ozone generated, the power used and the speed of killing vegetative cells. The surface temperature during plasma generation is also higher in the case of FR4. An inoculated FR4 or SC device produces less ozone than the respective clean devices. Temperature studies show that the surface temperatures reached during plasma generation are in the range of 30°C–66°C (for FR4) and 20°C–49°C (for SC). Surface temperatures during plasma generation of inoculated devices are lower than the corresponding temperatures of clean devices. pH studies indicate a slight reduction in pH value due to plasma generation, which implies that while temperature and acidification may play a minor role in DBD plasma sterilization, the presence of the liquid on the dielectric surface hampers sterilization and as the liquid evaporates, sterilization improves. PMID:23951023

Effect of dielectric and liquid on plasma sterilization using dielectric barrier discharge plasma.

PubMed

Mastanaiah, Navya; Johnson, Judith A; Roy, Subrata

2013-01-01

Plasma sterilization offers a faster, less toxic and versatile alternative to conventional sterilization methods. Using a relatively small, low temperature, atmospheric, dielectric barrier discharge surface plasma generator, we achieved ≥ 6 log reduction in concentration of vegetative bacterial and yeast cells within 4 minutes and ≥ 6 log reduction of Geobacillus stearothermophilus spores within 20 minutes. Plasma sterilization is influenced by a wide variety of factors. Two factors studied in this particular paper are the effect of using different dielectric substrates and the significance of the amount of liquid on the dielectric surface. Of the two dielectric substrates tested (FR4 and semi-ceramic (SC)), it is noted that the FR4 is more efficient in terms of time taken for complete inactivation. FR4 is more efficient at generating plasma as shown by the intensity of spectral peaks, amount of ozone generated, the power used and the speed of killing vegetative cells. The surface temperature during plasma generation is also higher in the case of FR4. An inoculated FR4 or SC device produces less ozone than the respective clean devices. Temperature studies show that the surface temperatures reached during plasma generation are in the range of 30°C-66 °C (for FR4) and 20 °C-49 °C (for SC). Surface temperatures during plasma generation of inoculated devices are lower than the corresponding temperatures of clean devices. pH studies indicate a slight reduction in pH value due to plasma generation, which implies that while temperature and acidification may play a minor role in DBD plasma sterilization, the presence of the liquid on the dielectric surface hampers sterilization and as the liquid evaporates, sterilization improves.

Device for generation of pulsed corona discharge

DOEpatents

Gutsol, Alexander F [San Ramon, CA; Fridman, Alexander [Marlton, NJ; Blank, Kenneth [Philadelphia, PA; Korobtsev, Sergey [Moscow, RU; Shiryaevsky, Valery [Moscow, RU; Medvedev, Dmitry [Moscow, RU

2012-05-08

The invention is a method and system for the generation of high voltage, pulsed, periodic corona discharges capable of being used in the presence of conductive liquid droplets. The method and system can be used, for example, in different devices for cleaning of gaseous or liquid media using pulsed corona discharge. Specially designed electrodes and an inductor increase the efficiency of the system, permit the plasma chemical oxidation of detrimental impurities, and increase the range of stable discharge operations in the presence of droplets of water or other conductive liquids in the discharge chamber.

Simulation of dust voids in complex plasmas

NASA Astrophysics Data System (ADS)

Goedheer, W. J.; Land, V.

2008-12-01

In dusty radio-frequency (RF) discharges under micro-gravity conditions often a void is observed, a dust free region in the discharge center. This void is generated by the drag of the positive ions pulled out of the discharge by the electric field. We have developed a hydrodynamic model for dusty RF discharges in argon to study the behaviour of the void and the interaction between the dust and the plasma background. The model is based on a recently developed theory for the ion drag force and the charging of the dust. With this model, we studied the plasma inside the void and obtained an understanding of the way it is sustained by heat generated in the surrounding dust cloud. When this heating mechanism is suppressed by lowering the RF power, the plasma density inside the void decreases, even below the level where the void collapses, as was recently shown in experiments on board the International Space Station. In this paper we present results of simulations of this collapse. At reduced power levels the collapsed central cloud behaves as an electronegative plasma with corresponding low time-averaged electric fields. This enables the creation of relatively homogeneous Yukawa balls, containing more than 100 000 particles. On earth, thermophoresis can be used to balance gravity and obtain similar dust distributions.

Electric discharge microplasmas generated in highly fluctuating fluids: Characteristics and application to the synthesis of molecular diamond

NASA Astrophysics Data System (ADS)

Stauss, Sven

2014-10-01

Plasma-based fabrication of novel nanomaterials and nanostructures is paramount for the development of next-generation electronic devices and for green energy applications. In particular, controlling the interactions between plasmas and materials interfaces, and the plasma fluctuations are crucial for further development of plasma-based processes and bottom-up growth of nanomaterials. Discharge microplasmas generated in supercritical fluids represent a special class of high-pressure plasmas, where fluctuations on the molecular scale influence the discharge properties and the possible bottom-up growth of nanomaterials. In the first part of the talk, we will discuss an anomaly observed for microplasmas generated near the critical point, a local decrease in the breakdown voltage, which has been observed for both molecular and monoatomic gases. This anomalous behavior is suggested to be caused by the concomitant decrease of the ionization potential due to the formation of clusters near the critical point, and the formation of extended electron mean free paths induced by the high-density fluctuation near the critical point. We will also show that when generating microplasma discharges close to the critical point, that the high-density fluctuation of the supercritical fluid persists. In the second part of the presentation, we will first introduce the basic properties of diamondoids and their potential for application in many different fields - biotechnology, medicine, opto- and nanoelectronics - before discussing their synthesis by microplasmas generated inside both conventional batch-type and continuous flow reactors, using the smallest diamondoid, adamantane, as a precursor and seed. Finally we show that one possible growth mechanism of larger diamondoids from smaller ones consists in the repeated abstraction of hydrogen terminations and the addition of methyl radicals. Supported financially in part by Grant No. 23760688 and Grant No. 21110002 from the Ministry of Education, Culture, Sports, Science and Technology of Japan.

Generation of warm dense matter using an argon based capillary discharge laser

NASA Astrophysics Data System (ADS)

Rossall, A. K.; Tallents, G. J.

2015-06-01

Argon based capillary discharge lasers operating in the extreme ultra violet (EUV) at 46.9 nm with output up to 0.5 mJ energy per pulse and repetition rates up to 10 Hz are capable of focused irradiances of 109-1012 W cm-2 and can be used to generate plasma in the warm dense matter regime by irradiating solid material. To model the interaction between such an EUV laser and solid material, the 2D radiative-hydrodynamic code POLLUX has been modified to include absorption via direct photo-ionisation, a super-configuration model to describe the ionization-dependent electronic configurations and a calculation of plasma refractive indices for ray tracing of the incident EUV laser radiation. A simulation study is presented, demonstrating how capillary discharge lasers of 1200 ps pulse duration can be used to generate warm dense matter at close to solid densities with temperatures of a few eV and energy densities up to 1 × 105 J cm-3. Plasmas produced by EUV laser irradiation are shown to be useful for examining the properties of warm dense matter as, for example, plasma emission is not masked by hotter, less dense plasma emission that occurs with visible/infra-red laser target irradiation.

Pulsed plasma thruster by applied a high current hollow cathode discharge

NASA Astrophysics Data System (ADS)

Watanabe, Masayuki; N. Nogera Team; T. Kamada Team

2013-09-01

The pulsed plasma thruster applied by a high current hollow cathode discharge has been investigated. In this research, the pseudo-spark discharge (PSD), which is a one of a pulsed high current hollow cathode discharge, is applied to the plasma thruster. In PSD, the opposite surfaces of the anode and cathode have a small circular hole and the cathode has a cylindrical cavity behind the circular hole. To generate the high speed plasma flow, the diameter of the anode hole is enlarged as compared with that of the cathode hole. As a result, the plasma is accelerated by a combination of an electro-magnetic force and a thermo-dynamic force inside a cathode cavity. For the improvement of the plasma jet characteristic, the magnetic field is also applied to the plasma jet. To magnetize the plasma jet, the external magnetic field is directly induced nearby the electrode holes. Consequently, the plasma jet is accelerated with the self-azimuthal magnetic field. With the magnetic field, the temperature and the density of the plasma jet were around 5 eV and in the order of 10 19 m-3. The density increased several times as compared with that without the magnetic field.

Production of high transient heat and particle fluxes in a linear plasma device

NASA Astrophysics Data System (ADS)

De Temmerman, G.; Zielinski, J. J.; van der Meiden, H.; Melissen, W.; Rapp, J.

2010-08-01

We report on the generation of high transient heat and particle fluxes in a linear plasma device by pulsed operation of the plasma source. A capacitor bank is discharged into the source to transiently increase the discharge current up to 1.7 kA, allowing peak densities and temperature of 70×1020 m-3 and 6 eV corresponding to a surface power density of about 400 MW m-2.

Transfer of a cold atmospheric pressure plasma jet through a long flexible plastic tube

NASA Astrophysics Data System (ADS)

Kostov, Konstantin G.; Machida, Munemasa; Prysiazhnyi, Vadym; Honda, Roberto Y.

2015-04-01

This work proposes an experimental configuration for the generation of a cold atmospheric pressure plasma jet at the downstream end of a long flexible plastic tube. The device consists of a cylindrical dielectric chamber where an insulated metal rod that serves as high-voltage electrode is inserted. The chamber is connected to a long (up to 4 m) commercial flexible plastic tube, equipped with a thin floating Cu wire. The wire penetrates a few mm inside the discharge chamber, passes freely (with no special support) along the plastic tube and terminates a few millimeters before the tube end. The system is flushed with Ar and the dielectric barrier discharge (DBD) is ignited inside the dielectric chamber by a low frequency ac power supply. The gas flow is guided by the plastic tube while the metal wire, when in contact with the plasma inside the DBD reactor, acquires plasma potential. There is no discharge inside the plastic tube, however an Ar plasma jet can be extracted from the downstream tube end. The jet obtained by this method is cold enough to be put in direct contact with human skin without an electric shock. Therefore, by using this approach an Ar plasma jet can be generated at the tip of a long plastic tube far from the high-voltage discharge region, which provides the safe operation conditions and device flexibility required for medical treatment.

Study of surface atmospheric pressure glow discharge plasma based on ultrathin laminated electrodes in air

NASA Astrophysics Data System (ADS)

Zhao, Luxiang; Liu, Wenzheng; Li, Zhiyi; Ma, Chuanlong

2018-05-01

A method to generate large-area surface plasma in air by micro-discharge is proposed. Two ultrathin laminated electrode structures of non-insulating and insulating types were formed by using the nanoscale ITO conductive layer. The surface glow discharge in atmospheric air is realized in low discharge voltage by constructing the special electric field of two-dimensional unidirectional attenuation. In particular, the insulating electrode structure can avoid the loss of ITO electrodes so that the discharge stability can be increased, and the treated objects can be prevented from metal ion pollution caused by the electrode in the discharge. It has broad application prospects in the fields of aerodynamics and material surface treatment.

Novel high-frequency energy-efficient pulsed-dc generator for capacitively coupled plasma discharge

NASA Astrophysics Data System (ADS)

Mamun, Md Abdullah Al; Furuta, Hiroshi; Hatta, Akimitsu

2018-03-01

The circuit design, assembly, and operating tests of a high-frequency and high-voltage (HV) pulsed dc generator (PDG) for capacitively coupled plasma (CCP) discharge inside a vacuum chamber are reported. For capacitive loads, it is challenging to obtain sharp rectangular pulses with fast rising and falling edges, requiring intense current for quick charging and discharging. The requirement of intense current generally limits the pulse operation frequency. In this study, we present a new type of PDG consisting of a pair of half-resonant converters and a constant current-controller circuit connected with HV solid-state power switches that can deliver almost rectangular high voltage pulses with fast rising and falling edges for CCP discharge. A prototype of the PDG is assembled to modulate from a high-voltage direct current (HVdc) input into a pulsed HVdc output, while following an input pulse signal and a set current level. The pulse rise time and fall time are less than 500 ns and 800 ns, respectively, and the minimum pulse width is 1 µs. The maximum voltage for a negative pulse is 1000 V, and the maximum repetition frequency is 500 kHz. During the pulse on time, the plasma discharge current is controlled steadily at the set value. The half-resonant converters in the PDG perform recovery of the remaining energy from the capacitive load at every termination of pulse discharge. The PDG performed with a high energy efficiency of 85% from the HVdc input to the pulsed dc output at a repetition rate of 1 kHz and with stable plasma operation in various discharge conditions. The results suggest that the developed PDG can be considered to be more efficient for plasma processing by CCP.

Novel high-frequency energy-efficient pulsed-dc generator for capacitively coupled plasma discharge.

PubMed

Mamun, Md Abdullah Al; Furuta, Hiroshi; Hatta, Akimitsu

2018-03-01

The circuit design, assembly, and operating tests of a high-frequency and high-voltage (HV) pulsed dc generator (PDG) for capacitively coupled plasma (CCP) discharge inside a vacuum chamber are reported. For capacitive loads, it is challenging to obtain sharp rectangular pulses with fast rising and falling edges, requiring intense current for quick charging and discharging. The requirement of intense current generally limits the pulse operation frequency. In this study, we present a new type of PDG consisting of a pair of half-resonant converters and a constant current-controller circuit connected with HV solid-state power switches that can deliver almost rectangular high voltage pulses with fast rising and falling edges for CCP discharge. A prototype of the PDG is assembled to modulate from a high-voltage direct current (HVdc) input into a pulsed HVdc output, while following an input pulse signal and a set current level. The pulse rise time and fall time are less than 500 ns and 800 ns, respectively, and the minimum pulse width is 1 µs. The maximum voltage for a negative pulse is 1000 V, and the maximum repetition frequency is 500 kHz. During the pulse on time, the plasma discharge current is controlled steadily at the set value. The half-resonant converters in the PDG perform recovery of the remaining energy from the capacitive load at every termination of pulse discharge. The PDG performed with a high energy efficiency of 85% from the HVdc input to the pulsed dc output at a repetition rate of 1 kHz and with stable plasma operation in various discharge conditions. The results suggest that the developed PDG can be considered to be more efficient for plasma processing by CCP.

PLASMA DEVICE

DOEpatents

Baker, W.R.

1961-08-22

A device is described for establishing and maintaining a high-energy, rotational plasma for use as a fast discharge capacitor. A disc-shaped, current- conducting plasma is formed in an axinl magnetic field and a crossed electric field, thereby creating rotational kinetic enengy in the plasma. Such energy stored in the rotation of the plasma disc is substantial and is convertible tc electrical energy by generator action in an output line electrically coupled to the plasma volume. Means are then provided for discharging the electrical energy into an external circuit coupled to the output line to produce a very large pulse having an extremely rapid rise time in the waveform thereof. (AE C)

Reproducing continuous radio blackout using glow discharge plasma

DOE Office of Scientific and Technical Information (OSTI.GOV)

Xie, Kai; Li, Xiaoping; Liu, Donglin

2013-10-15

A novel plasma generator is described that offers large-scale, continuous, non-magnetized plasma with a 30-cm-diameter hollow structure, which provides a path for an electromagnetic wave. The plasma is excited by a low-pressure glow discharge, with varying electron densities ranging from 10{sup 9} to 2.5 × 10{sup 11} cm{sup −3}. An electromagnetic wave propagation experiment reproduced a continuous radio blackout in UHF-, L-, and S-bands. The results are consistent with theoretical expectations. The proposed method is suitable in simulating a plasma sheath, and in researching communications, navigation, electromagnetic mitigations, and antenna compensation in plasma sheaths.

A Guillemin type E pulse forming network as the driver for a pulsed, high density plasma source.

PubMed

Rathod, Priyavandna J; Anitha, V P; Sholapurwala, Z H; Saxena, Y C

2014-06-01

A Guillemin type E pulse forming network (PFN) has been designed, developed, and tested for its application in generating high density (~1 × 10(18) m(-3)) plasmas. In the present study, plasma thus generated is utilized to investigate the interaction of high power microwaves (HPMs) with plasma in an experimental architecture known as SYMPLE (System for Microwave PLasma Experiment). Plasma discharges of ~100 μs (max) duration are to be produced, by delivering energy of 5 kJ stored in a PFN to the plasma source, a washer gun. The output of the PFN, in terms of its rise time, flat top and amplitude, needs to be tailored, depending on the experimental requirements. An ignitron (NL8900) trigger generator (ITG) is developed in-house to control the PFN discharge through the gun. This ITG is also to be used in a circuit that synchronizes the HPM and plasma shots, to ensure that HPM-plasma interaction takes place during a temporal regime where appropriate parametric conditions are satisfied. Hence it is necessary to retain the jitter within ±2.5 μs. Further, requirement on plasma quiescence (~10%) necessitates maintaining the ripple within 5%. The developmental work of the PFN, keeping in view the above criteria and the test results, is presented in this paper. The parameters of the PFN have been analytically approximated and verified with PSPICE simulation. The test results presented include rise time ~5-8 μs, flat top variable in the range 20-100 μs, ripple within ~1.5%, and jitter within ±2.5 μs, producing quiescent (<10%) plasma discharge meeting the experimental requirements.

Modeling polyvinyl chloride Plasma Modification by Neural Networks

NASA Astrophysics Data System (ADS)

Wang, Changquan

2018-03-01

Neural networks model were constructed to analyze the connection between dielectric barrier discharge parameters and surface properties of material. The experiment data were generated from polyvinyl chloride plasma modification by using uniform design. Discharge voltage, discharge gas gap and treatment time were as neural network input layer parameters. The measured values of contact angle were as the output layer parameters. A nonlinear mathematical model of the surface modification for polyvinyl chloride was developed based upon the neural networks. The optimum model parameters were obtained by the simulation evaluation and error analysis. The results of the optimal model show that the predicted value is very close to the actual test value. The prediction model obtained here are useful for discharge plasma surface modification analysis.

Dielectric barrier discharges: progress on plasma sources and on the understanding of regimes and single filaments

NASA Astrophysics Data System (ADS)

Brandenburg, Ronny

2017-05-01

Dielectric barrier discharges (DBDs) are plasmas generated in configurations with an insulating (dielectric) material between the electrodes which is responsible for a self-pulsing operation. DBDs are a typical example of nonthermal atmospheric or normal pressure gas discharges. Initially used for the generation of ozone, they have opened up many other fields of application. Therefore DBDs are a relevant tool in current plasma technology as well as an object for fundamental studies. Another motivation for further research is the fact that so-called partial discharges in insulated high voltage systems are special types of DBDs. The breakdown processes, the formation of structures, and the role of surface processes are currently under investigation. This review is intended to give an update to the already existing literature on DBDs considering the research and development within the last two decades. The main principles and different modes of discharge generation are summarized. A collection of known as well as special electrode configurations and reactor designs will be presented. This shall demonstrate the different and broad possibilities, but also the similarities and common aspects of devices for different fields of applications explored within the last years. The main part is devoted to the progress on the investigation of different aspects of breakdown and plasma formation with the focus on single filaments or microdischarges. This includes a summary of the current knowledge on the electrical characterization of filamentary DBDs. In particular, the recent new insights on the elementary volume and surface memory mechanisms in these discharges will be discussed. An outlook for the forthcoming challenges on research and development will be given.

Glow plasma trigger for electron cyclotron resonance ion sources.

PubMed

Vodopianov, A V; Golubev, S V; Izotov, I V; Nikolaev, A G; Oks, E M; Savkin, K P; Yushkov, G Yu

2010-02-01

Electron cyclotron resonance ion sources (ECRISs) are particularly useful for nuclear, atomic, and high energy physics, as unique high current generators of multicharged ion beams. Plasmas of gas discharges in an open magnetic trap heated by pulsed (100 micros and longer) high power (100 kW and higher) high-frequency (greater than 37.5 GHz) microwaves of gyrotrons is promising in the field of research in the development of electron cyclotron resonance sources for high charge state ion beams. Reaching high ion charge states requires a decrease in gas pressure in the magnetic trap, but this method leads to increases in time, in which the microwave discharge develops. The gas breakdown and microwave discharge duration becomes greater than or equal to the microwave pulse duration when the pressure is decreased. This makes reaching the critical plasma density initiate an electron cyclotron resonance (ECR) discharge during pulse of microwave gyrotron radiation with gas pressure lower than a certain threshold. In order to reduce losses of microwave power, it is necessary to shorten the time of development of the ECR discharge. For fast triggering of ECR discharge under low pressure in an ECRIS, we initially propose to fill the magnetic trap with the plasmas of auxiliary pulsed discharges in crossed ExB fields. The glow plasma trigger of ECR based on a Penning or magnetron discharge has made it possible not only to fill the trap with plasma with density of 10(12) cm(-3), required for a rapid increase in plasma density and finally for ECR discharge ignition, but also to initially heat the plasma electrons to T(e) approximately = 20 eV.

Methods and Apparatus for Pulsed-DC Dielectric Barrier Discharge Plasma Actuator and Circuit

NASA Technical Reports Server (NTRS)

Corke, Thomas C. (Inventor); Gold, Calman (Inventor); Kaszeta, Richard (Inventor)

2017-01-01

A plasma generating device intended to induce a flow in a fluid via plasma generation includes a dielectric separating two electrodes and a power supply. The first electrode is exposed to a fluid flow while the second electrode is positioned under the dielectric. The power supply is electrically coupled to a switch and the first and second electrodes. When the power supply is energized by repeated action of the switch, it causes a pulsed DC current between the electrodes which causes the fluid to ionize generating a plasma. The generation of the plasma induces a force with a velocity component in the fluid.

Preliminary Experiment of Non-Inductive Plasma Current Startup in SUNIST Spherical Tokamak

NASA Astrophysics Data System (ADS)

He, Yexi; Zhang, Liang; Xie, Lifeng; Tang, Yi; Yang, Xuanzong; Feng, Chunhua; Fu, Hongjun

2006-01-01

The non-inductive plasma current startup is an important motivation in SUNIST spherical tokamak. In the recent experiment, the magnetron microwave system of 100 kW and 2.45 GHz has been used to the ECR plasma current startup. Besides the toroidal field, a vertical field was applied to generate preliminary toroidal plasma current without the action of the central solenoid. As the evidence of plasma current startup with the effect of vertical field drift, the direction of plasma current is changed when the direction of vertical field changes during the ECR plasma current startup discharge. We also observed a maximum plasma current by scanning vertical field in both directions. Additionally, we used electrode discharge to assist the ECR plasma current startup.

Experimental investigation and numerical modelling of positive corona discharge: ozone generation

NASA Astrophysics Data System (ADS)

Yanallah, K; Pontiga, F; Fernández-Rueda, A; Castellanos, A

2009-03-01

The spatial distribution of the species generated in a wire-cylinder positive corona discharge in pure oxygen has been computed using a plasma chemistry model that includes the most significant reactions between electrons, ions, atoms and molecules. The plasma chemistry model is included in the continuity equations of each species, which are coupled with Poisson's equation for the electric field and the energy conservation equation for the gas temperature. The current-voltage characteristic measured in the experiments has been used as an input data to the numerical simulation. The numerical model is able to reproduce the basic structure of the positive corona discharge and highlights the importance of Joule heating on ozone generation. The average ozone density has been computed as a function of current intensity and compared with the experimental measurements of ozone concentration determined by UV absorption spectroscopy.

Self-similar magnetohydrodynamic model for direct current discharge fireball experiments

NASA Astrophysics Data System (ADS)

Tsui, K. H.; Navia, C. E.; Robba, M. B.; Carneiro, L. T.; Emelin, S. E.

2006-11-01

Ball lightning models and corresponding laboratory efforts in generating fireballs are briefly summarized to give an overview of the current status. In particular, emphasis is given to direct current discharge experiments at atmospheric pressure such as capillary discharge with a plasma plume in front of the anode opening [Emelin et al., Tech. Phys. Letters 23, 758 (1997)] and water resistor discharge with fluttering fireball overhead [Egorov and Stepanov, Tech. Phys. 47, 1584 (2002)]. These fireballs are interpreted as laboratory demonstrations of the self-similar magnetohydrodynamic (MHD) model of ball lightning [Tsui, Phys. Plasmas 13, 072102 (2006)].

Modelling chemical reactions in dc plasma inside oxygen bubbles in water

NASA Astrophysics Data System (ADS)

Takeuchi, N.; Ishii, Y.; Yasuoka, K.

2012-02-01

Plasmas generated inside oxygen bubbles in water have been developed for water purification. Zero-dimensional numerical simulations were used to investigate the chemical reactions in plasmas driven by dc voltage. The numerical and experimental results of the concentrations of hydrogen peroxide and ozone in the solution were compared with a discharge current between 1 and 7 mA. Upon increasing the water vapour concentration inside bubbles, we saw from the numerical results that the concentration of hydrogen peroxide increased with discharge current, whereas the concentration of ozone decreased. This finding agreed with the experimental results. With an increase in the discharge current, the heat flux from the plasma to the solution increased, and a large amount of water was probably vaporized into the bubbles.

Experimental investigation on the effect of plasma jet in the triggered discharge process of a gas switch

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tie, W., E-mail: twh.110.666@163.com, E-mail: 84470220@qq.com; Xi'an Jiaotong University, Xi'an 710049; Liu, S.

The temporal and spatial evolution of a plasma jet generated by a spark discharge was observed. The electron temperature and density were obtained under different time and gas pressures by optical emission spectroscopy. Moreover, the discharge process of the plasma-jet triggered gas switch was recorded and analyzed at the lowest working coefficient. The results showed that the plasma jet moved forward in a bullet mode, and the advancing velocity increased with the decrease of pressure, and decreased with time growing. At initial time, the maximum velocity of a plasma jet could reach 3.68 × 10{sup 6 }cm/s. The electron temperature decreased from 2.0 eVmore » to 1.3 eV, and the electron density increased from 3.1 × 10{sup 15}/cm{sup 3} to 6.3 × 10{sup 15}/cm{sup 3} at the initial moment as the gas pressure increases from 0.1 MPa to 0.32 MPa. For a two-gap gas switch, the discharge performances were more depended on the second discharge spark gap (gap 2). Because plasma jet promoted the discharge in Gap 2, the gas switch operating in mode II had better triggered discharge characteristics. In the discharge process, the plasma-jet triggering had the effect of non-penetrating inducing, which not only provided initial electrons for reducing statistical lag but also enhanced the local electric field. The discharge was initiated and accelerated from electron avalanche to streamer. Therefore, a fast discharge was occurred in the gas switch.« less

Heating and cooling of the multiply charged ion nonequilibrium plasma in a high-current extended low-inductance discharge

NASA Astrophysics Data System (ADS)

Burtsev, V. A.; Kalinin, N. V.

2014-09-01

Using a radiation magnetohydrodynamics two-temperature model (RMHD model) of a high-current volumetric radiating Z-discharge, the heating and cooling of the nitrogen plasma in a pulsed pinched extended discharge is investigated as applied to the problem of creating a recombination laser based on 3 → 2 transitions of hydrogen-like nitrogen ions (λ = 13.4 nm). It is shown that the power supply of the discharge, which is represented by a dual storage-forming line and a transmission line, makes it possible to raise the power density of the nitrogen plasma to 0.01-1.00 TW/cm3. Accordingly, there arises the possibility of generating a fully ionized (i.e., consisting of bare nuclei and electrons) plasma through the heating (compression) of electrons owing to the self-magnetic field of the plasma current and Joule heat even if the plasma is cooled by its own radiation at this stage. Such a plasma is needed to produce the lasing (active) medium of a recombination laser based on electron transitions in hydrogen-like ions. At the second stage, it is necessary to rapidly and deeply cool the plasma to 20-40 eV for 1-2 ns. Cooling of the fully ionized expanding plasma was numerically simulated with the discharge current switched on and off by means of a switch with a rapidly rising resistance. In both cases, the plasma expansion in the discharge is not adiabatic. Even after the discharge current is fairly rapidly switched off, heating of electrons continues inside the plasma column for a time longer than the switching time. Discharge current switchoff improves the electron cooling efficiency only slightly. Under such conditions, the plasma cools down to 50-60 eV in the former case and to 46-54 eV in the latter case for 2-3 ns.

Nitric Oxide Studies in Low Temperature Plasmas Generated with a Nanosecond Pulse Sphere Gap Electrical Discharge

NASA Astrophysics Data System (ADS)

Burnette, David Dean

This dissertation presents studies of NO kinetics in a plasma afterglow using various nanosecond pulse discharges across a sphere gap. The discharge platform is developed to produce a diffuse plasma volume large enough to allow for laser diagnostics in a plasma that is rich in vibrationally-excited molecules. This plasma is characterized by current and voltage traces as well as ICCD and NO PLIF images that are used to monitor the plasma dimensions and uniformity. Temperature and vibrational loading measurements are performed via coherent anti-Stokes Raman spectroscopy (CARS). Absolute NO concentrations are obtained by laser-induce fluorescence (LIF) measurements, and N and O densities are found using two photon absorption laser-induced fluorescence (TALIF). For all dry air conditions studied, the NO behavior is characterized by a rapid rate of formation consistent with an enhanced Zeldovich process involving electronically-excited nitrogen species that are generated within the plasma. After several microseconds, the NO evolution is entirely controlled by the reverse Zeldovich process. These results show that under the chosen range of conditions and even in extreme instances of vibrational loading, there is no formation channel beyond ~2 musec. Both the NO formation and consumption mechanisms are strongly affected by the addition of fuel species, producing much greater NO concentrations in the afterglow.

Generation conditions of CW Diode Laser Sustained Plasma

NASA Astrophysics Data System (ADS)

Nishimoto, Koji; Matsui, Makoto; Ono, Takahiro

2016-09-01

Laser sustained plasma was generated using 1 kW class continuous wave diode laser. The laser beam was focused on the seed plasma generated by arc discharge in 1 MPa xenon lamp. The diode laser has advantages of high energy conversion efficiency of 80%, ease of maintenance, compact size and availability of conventional quartz based optics. Therefore, it has a prospect of further development compared with conventional CO2 laser. In this study, variation of the plasma shape caused by laser power is observed and also temperature distribution in the direction of plasma radius is measured by optical emission spectroscopy.

Influence of ionic liquid and ionic salt on protein against the reactive species generated using dielectric barrier discharge plasma.

PubMed

Attri, Pankaj; Sarinont, Thapanut; Kim, Minsup; Amano, Takaaki; Koga, Kazunori; Cho, Art E; Choi, Eun Ha; Shiratani, Masaharu

2015-12-10

The presence of salts in biological solution can affect the activity of the reactive species (RS) generated by plasma, and so they can also have an influence on the plasma-induced sterilization. In this work, we assess the influence that diethylammonium dihydrogen phosphate (DEAP), an ionic liquid (IL), and sodium chloride (NaCl), an ionic salt (IS), have on the structural changes in hemoglobin (Hb) in the presence of RS generated using dielectric barrier discharge (DBD) plasma in the presence of various gases [O2, N2, Ar, He, NO (10%) + N2 and Air]. We carry out fluorescence spectroscopy to verify the generation of (•)OH with or without the presence of DEAP IL and IS, and we use electron spin resonance (ESR) to check the generation of H(•) and (•)OH. In addition, we verified the structural changes in the Hb structure after treatment with DBD in presence and absence of IL and IS. We then assessed the structural stability of the Hb in the presence of IL and IS by using molecular dynamic (MD) simulations. Our results indicate that the IL has a strong effect on the conservation of the Hb structure relative to that of IS against RS generated by plasma.

Influence of ionic liquid and ionic salt on protein against the reactive species generated using dielectric barrier discharge plasma

NASA Astrophysics Data System (ADS)

Attri, Pankaj; Sarinont, Thapanut; Kim, Minsup; Amano, Takaaki; Koga, Kazunori; Cho, Art E.; Ha Choi, Eun; Shiratani, Masaharu

2015-12-01

The presence of salts in biological solution can affect the activity of the reactive species (RS) generated by plasma, and so they can also have an influence on the plasma-induced sterilization. In this work, we assess the influence that diethylammonium dihydrogen phosphate (DEAP), an ionic liquid (IL), and sodium chloride (NaCl), an ionic salt (IS), have on the structural changes in hemoglobin (Hb) in the presence of RS generated using dielectric barrier discharge (DBD) plasma in the presence of various gases [O2, N2, Ar, He, NO (10%) + N2 and Air]. We carry out fluorescence spectroscopy to verify the generation of •OH with or without the presence of DEAP IL and IS, and we use electron spin resonance (ESR) to check the generation of H• and •OH. In addition, we verified the structural changes in the Hb structure after treatment with DBD in presence and absence of IL and IS. We then assessed the structural stability of the Hb in the presence of IL and IS by using molecular dynamic (MD) simulations. Our results indicate that the IL has a strong effect on the conservation of the Hb structure relative to that of IS against RS generated by plasma.

Advances in electron kinetics and theory of gas discharges

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kolobov, Vladimir I.; The University of Alabama in Huntsville, Huntsville, Alabama 35899

2013-10-15

“Electrons, like people, are fertile and infertile: high-energy electrons are fertile and able to reproduce.”—Lev TsendinModern physics of gas discharges increasingly uses physical kinetics for analysis of non-equilibrium plasmas. The description of underlying physics at the kinetic level appears to be important for plasma applications in modern technologies. In this paper, we attempt to grasp the legacy of Professor Lev Tsendin, who advocated the use of the kinetic approach for understanding fundamental problems of gas discharges. We outline the fundamentals of electron kinetics in low-temperature plasmas, describe elements of the modern kinetic theory of gas discharges, and show examples ofmore » the theoretical approach to gas discharge problems used by Lev Tsendin. Important connections between electron kinetics in gas discharges and semiconductors are also discussed. Using several examples, we illustrate how Tsendin's ideas and methods are currently being developed for the implementation of next generation computational tools for adaptive kinetic-fluid simulations of gas discharges used in modern technologies.« less

Method and apparatus for charged particle propagation

DOEpatents

Hershcovitch, A.

1996-11-26

A method and apparatus are provided for propagating charged particles from a vacuum to a higher pressure region. A generator includes an evacuated chamber having a gun for discharging a beam of charged particles such as an electron beam or ion beam. The beam is discharged through a beam exit in the chamber into a higher pressure region. A plasma interface is disposed at the beam exit and includes a plasma channel for bounding a plasma maintainable between a cathode and an anode disposed at opposite ends thereof. The plasma channel is coaxially aligned with the beam exit for propagating the beam from the chamber, through the plasma, and into the higher pressure region. The plasma is effective for pumping down the beam exit for preventing pressure increase in the chamber and provides magnetic focusing of the beam discharged into the higher pressure region 24. 7 figs.

Bio-Decontamination of Water and Surfaces by DC Discharges in Atmospheric Air

NASA Astrophysics Data System (ADS)

Machala, Zdenko; Tarabová, Barbora; Pelach, Michal; Šipoldová, Zuzana; Hensel, Karol; Janda, Mário; Šikurová, Libuša

Two types of DC-driven atmospheric air discharges, including a streamer corona and a transient spark with short high current pulses of limited energy, were employed for bio-decontamination of water and various surfaces (agar plates, plastic foils, human teeth) contaminated by bacteria or spores (Salmonella typhimurium, Bacillus cereus). Both discharges generate cold non-equilibrium plasma. The discharges combined with the electro-spraying of the treated water through the needle electrode lead to fast and efficient bio-decontamination. Experiments comparing direct and indirect plasma effects, oxidation stress measurements in the cell membranes, and chemical changes induced in the treated water enable assessment of the plasma agents being responsible for microbial inactivation. Radicals and reactive oxygen species seem to be dominant biocidal agents, although deeper understanding of the plasma-induced water chemistry and of the temporal evolution of the bio-inactivation processes is needed.

Ion beam generating apparatus

DOEpatents

Brown, I.G.; Galvin, J.

1987-12-22

An ion generating apparatus utilizing a vacuum chamber, a cathode and an anode in the chamber. A source of electrical power produces an arc or discharge between the cathode and anode. The arc is sufficient to vaporize a portion of the cathode to form a plasma. The plasma is directed to an extractor which separates the electrons from the plasma, and accelerates the ions to produce an ion beam. 10 figs.

Laser beam coupling with capillary discharge plasma for laser wakefield acceleration applications

NASA Astrophysics Data System (ADS)

Bagdasarov, G. A.; Sasorov, P. V.; Gasilov, V. A.; Boldarev, A. S.; Olkhovskaya, O. G.; Benedetti, C.; Bulanov, S. S.; Gonsalves, A.; Mao, H.-S.; Schroeder, C. B.; van Tilborg, J.; Esarey, E.; Leemans, W. P.; Levato, T.; Margarone, D.; Korn, G.

2017-08-01

One of the most robust methods, demonstrated to date, of accelerating electron beams by laser-plasma sources is the utilization of plasma channels generated by the capillary discharges. Although the spatial structure of the installation is simple in principle, there may be some important effects caused by the open ends of the capillary, by the supplying channels etc., which require a detailed 3D modeling of the processes. In the present work, such simulations are performed using the code MARPLE. First, the process of capillary filling with cold hydrogen before the discharge is fired, through the side supply channels is simulated. Second, the simulation of the capillary discharge is performed with the goal to obtain a time-dependent spatial distribution of the electron density near the open ends of the capillary as well as inside the capillary. Finally, to evaluate the effectiveness of the beam coupling with the channeling plasma wave guide and of the electron acceleration, modeling of the laser-plasma interaction was performed with the code INF&RNO.

Plasma dynamics in a packed bed dielectric barrier discharge (DBD) operated in helium

NASA Astrophysics Data System (ADS)

Mujahid, Zaka-ul-Islam; Hala, Ahmed

2018-03-01

Packed bed dielectric barrier discharges (DBDs) are very promising for several applications including remediation of environmental pollutants and greenhouse gas conversion. In this work, we have investigated the space and time-resolved emission from a packed bed DBD operated in helium, to understand the plasma dynamics. We have chosen a simple planar DBD arrangement with a patterned dielectric, which mimics the spherical boundaries between the dielectric pellets and allows the optical access to the plasma. The results show that plasma is sustained in a packed bed DBD by three mechanisms: filamentary discharge in the void (between the center of dielectric structures and the opposite electrode), microdischarges at the contact points and surface ionization waves over the dielectric surface. It is observed that for most of the duration plasma is generated at the contact points between the dielectric structures.

23RD International Conference on Phenomena in Ionized Gases, Volume 3

DTIC Science & Technology

1998-12-01

discharges, and high pressure glows; arcs; high frequency discharges; ionospheric magnetospheric, and astrophysical plasmas; plasma diagnostic methods ...kf) in pulse reflectometry. Second, it different frequencies , and an Abel inversion is gives a quantitative model of the behaviour of the wave... design V method in the case of narrow mutual pitch of surface electrodes for high concentration ozone generation. 2. Experimental setup 20 The electrode

Coupled microwave ECR and radio-frequency plasma source for plasma processing

DOEpatents

Tsai, Chin-Chi; Haselton, Halsey H.

1994-01-01

In a dual plasma device, the first plasma is a microwave discharge having its own means of plasma initiation and control. The microwave discharge operates at electron cyclotron resonance (ECR), and generates a uniform plasma over a large area of about 1000 cm.sup.2 at low pressures below 0.1 mtorr. The ECR microwave plasma initiates the second plasma, a radio frequency (RF) plasma maintained between parallel plates. The ECR microwave plasma acts as a source of charged particles, supplying copious amounts of a desired charged excited species in uniform manner to the RF plasma. The parallel plate portion of the apparatus includes a magnetic filter with static magnetic field structure that aids the formation of ECR zones in the two plasma regions, and also assists in the RF plasma also operating at electron cyclotron resonance.

Coupled microwave ECR and radio-frequency plasma source for plasma processing

DOEpatents

Tsai, C.C.; Haselton, H.H.

1994-03-08

In a dual plasma device, the first plasma is a microwave discharge having its own means of plasma initiation and control. The microwave discharge operates at electron cyclotron resonance (ECR), and generates a uniform plasma over a large area of about 1000 cm[sup 2] at low pressures below 0.1 mtorr. The ECR microwave plasma initiates the second plasma, a radio frequency (RF) plasma maintained between parallel plates. The ECR microwave plasma acts as a source of charged particles, supplying copious amounts of a desired charged excited species in uniform manner to the RF plasma. The parallel plate portion of the apparatus includes a magnetic filter with static magnetic field structure that aids the formation of ECR zones in the two plasma regions, and also assists in the RF plasma also operating at electron cyclotron resonance. 4 figures.

Apparatus for the plasma destruction of hazardous gases

DOEpatents

Kang, M.

1995-02-07

A plasma cell for destroying hazardous gases is described. An electric-discharge cell having an electrically conducting electrode onto which an alternating high-voltage waveform is impressed and a dielectric barrier adjacent thereto, together forming a high-voltage electrode, generates self-terminating discharges throughout a volume formed between this electrode and a grounded conducting liquid electrode. The gas to be transformed is passed through this volume. The liquid may be flowed, generating thereby a renewable surface. Moreover, since hydrochloric and hydrofluoric acids may be formed from destruction of various chlorofluorocarbons in the presence of water, a conducting liquid may be selected which will neutralize these corrosive compounds. The gases exiting the discharge region may be further scrubbed if additional purification is required. 4 figs.

Apparatus for the plasma destruction of hazardous gases

DOEpatents

Kang, Michael

1995-01-01

A plasma cell for destroying hazardous gases. An electric-discharge cell having an electrically conducting electrode onto which an alternating high-voltage waveform is impressed and a dielectric barrier adjacent thereto, together forming a high-voltage electrode, generates self-terminating discharges throughout a volume formed between this electrode and a grounded conducting liquid electrode. The gas to be transformed is passed through this volume. The liquid may be flowed, generating thereby a renewable surface. Moreover, since hydrochloric and hydrofluoric acids may be formed from destruction of various chlorofluorocarbons in the presence of water, a conducting liquid may be selected which will neutralize these corrosive compounds. The gases exiting the discharge region may be further scrubbed if additional purification is required.

Investigation and control of the {{\\rm{O}}}_{3}- to {NO}-transition in a novel sub-atmospheric pressure dielectric barrier discharge

NASA Astrophysics Data System (ADS)

Bansemer, Robert; Schmidt-Bleker, Ansgar; van Rienen, Ursula; Weltmann, Klaus-Dieter

2017-06-01

A novel flow-driven dielectric barrier discharge concept is presented, which uses a Venturi pump to transfer plasma-generated reactive oxygen and nitrogen species from a sub-atmospheric pressure (200{--}600 {mbar}) discharge region to ambient pressure and can be operated with air. By adjusting the working pressure of the device, the plasma chemistry can be tuned continuously from an ozone ({{{O}}}3)-dominated mode to a nitrogen oxides ({{NO}}x)-only mode. The plasma source is characterized focusing on the mechanisms effecting this mode change. The composition of the device’s output gas was determined using Fourier-transform infrared spectroscopy. The results are correlated to measurements of discharge chamber pressure and temperature as well as of input power. It is found that the mode-change temperature can be controlled by the discharge chamber pressure. The source concept is capable of generating an {{NO}}x-dominated plasma chemistry at gas temperatures distinctly below 400 {{K}}. Through mixing of the processed gas stream with a second flow of pressurized air required for the operation of the Venturi pump, the resulting product gas stream remains close to room temperature. A reduced zero-dimensional reaction kinetics model with only seven reactions is capable of describing the observed pressure- and temperature-dependence of the {{{O}}}3 to {{NO}}x mode-change.

In situ CF3 Detection in Low Pressure Inductive Discharges by Fourier Transform Infrared Spectroscopy

NASA Technical Reports Server (NTRS)

Kim, J. S.; Cappelli, M. A.; Sharma, S. P.; Arnold, J. O. (Technical Monitor)

1998-01-01

The detection of CF(x) (x=1-3) radicals in low pressure discharges using source gases such as CF4 and CHF3 is of importance to the understanding of their chemical structure and relevance in plasma based etching processes. These radicals are known to contribute to the formation of fluorocarbon polymer films, which affect the selectivity and anisotropy of etching. In this study, we present preliminary results of the quantitative measurement of trifluoromethyl radicals, CF3, in low pressure discharges. The discharge studied here is an inductively (transformer) coupled plasma (ICP) source in the GEC reference cell, operating on pure CF4 at pressures ranging from 10 - 100 mTorr, This plasma source generates higher electron number densities at lower operating pressures than obtainable with the parallel-plate capacitively coupled version of the GEC reference cell. Also, this expanded operating regime is more relevant to new generations of industrial plasma reactors being used by the microelectronics industry. Fourier transform infrared (FTIR) spectroscopy is employed to observe the absorption band of CF3 radicals in the electronic ground state X2Al in the region of 1233-1270/cm. The spectrometer is equipped with a high sensitivity HgCdTe (MCT) detector and has a fixed resolution of 0.125/cm. The CF3 concentrations are measured for a range of operating pressures and discharge power levels.

Generation and Reduction of NOx on Air-Fed Ozonizers

NASA Astrophysics Data System (ADS)

Ehara, Yoshiyasu; Amemiya, Yusuke; Yamamoto, Toshiaki

A generation and reduction of NOx on air-fed ozonizers using a ferroelectric packed bed reactor have been experimentally investigated. The reactors packed with CaTiO3, SrTiO3 and BaTiO3 pellets are examined for ozone generation. An ac voltage is applied to the reactor to generate partial discharge. Ozone concentration and the different nitrogen oxides at downstream of the packed bed reactor were measured with UV absorption ozone monitor and a Fourier transform infrared spectroscope respectively. The dielectric constant of packed ferroelectric pellets influences the discharge characteristic, ozone and NOx generations are varied by the dielectric constant value. Focusing on a discharge pulse current and maximum discharge magnitude, the ferroelectric packed bed plasma reactors have been evaluated on nitrogen oxide and ozone generated concentrations.

Multiple current peaks in room-temperature atmospheric pressure homogenous dielectric barrier discharge plasma excited by high-voltage tunable nanosecond pulse in air

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yang, De-Zheng; Wang, Wen-Chun; Zhang, Shuai

2013-05-13

Room temperature homogenous dielectric barrier discharge plasma with high instantaneous energy efficiency is acquired by using nanosecond pulse voltage with 20-200 ns tunable pulse width. Increasing the voltage pulse width can lead to the generation of regular and stable multiple current peaks in each discharge sequence. When the voltage pulse width is 200 ns, more than 5 organized current peaks can be observed under 26 kV peak voltage. Investigation also shows that the organized multiple current peaks only appear in homogenous discharge mode. When the discharge is filament mode, organized multiple current peaks are replaced by chaotic filament current peaks.

Characteristics of electromagnetic interference generated during discharge of Mylar samples. [spacecraft-environment interaction simulation

NASA Technical Reports Server (NTRS)

Leung, P. L.

1984-01-01

This paper discusses the measurements of the electromagnetic interference (EMI) generated during discharges of Mylar samples. The two components of EMI, the conducted emission and the radiated emission, are characterized by the replacement current and the radiated RF spectrum respectively. The measured radiated RF spectra reveal important information on the source of the electromagnetic radiation. The possible sources are the replacement current pulse and the discharged generated plasma. The scaling of the amplitudes of the EMI, as a function of the area of the test sample, is also discussed.

Study of the Anatomy of the X-Ray and Neutron Production Scaling Laws in the Plasma Focus (Particle Energy Spectrum and Optimization Criteria).

DTIC Science & Technology

1979-11-01

plasma focus operations have been experimentally analyzed in terms of (A) The fine structure of the axial-current channel during maximum of compression. (B) Correlation coefficient, for neutron yield n (by D2 discharges) and the multiplicity of the electron beam pulses; (C) Different values of the electrode voltage. The current distribution near the axial plasma column during the explosive decay of the column has been monitored and correlated with the electron beam production. Plasma focus discharges by our mode of operation generate high-intensity

Helicon plasma generator-assisted surface conversion ion source for the production of H- ion beams at the Los Alamos Neutron Science Centera)

NASA Astrophysics Data System (ADS)

Tarvainen, O.; Rouleau, G.; Keller, R.; Geros, E.; Stelzer, J.; Ferris, J.

2008-02-01

The converter-type negative ion source currently employed at the Los Alamos Neutron Science Center (LANSCE) is based on cesium enhanced surface production of H- ion beams in a filament-driven discharge. In this kind of an ion source the extracted H- beam current is limited by the achievable plasma density which depends primarily on the electron emission current from the filaments. The emission current can be increased by increasing the filament temperature but, unfortunately, this leads not only to shorter filament lifetime but also to an increase in metal evaporation from the filament, which deposits on the H- converter surface and degrades its performance. Therefore, we have started an ion source development project focused on replacing these thermionic cathodes (filaments) of the converter source by a helicon plasma generator capable of producing high-density hydrogen plasmas with low electron energy. In our studies which have so far shown that the plasma density of the surface conversion source can be increased significantly by exciting a helicon wave in the plasma, and we expect to improve the performance of the surface converter H- ion source in terms of beam brightness and time between services. The design of this new source and preliminary results are presented, along with a discussion of physical processes relevant for H- ion beam production with this novel design. Ultimately, we perceive this approach as an interim step towards our long-term goal, combining a helicon plasma generator with an SNS-type main discharge chamber, which will allow us to individually optimize the plasma properties of the plasma cathode (helicon) and H- production (main discharge) in order to further improve the brightness of extracted H- ion beams.

Helicon plasma generator-assisted surface conversion ion source for the production of H(-) ion beams at the Los Alamos Neutron Science Center.

PubMed

Tarvainen, O; Rouleau, G; Keller, R; Geros, E; Stelzer, J; Ferris, J

2008-02-01

The converter-type negative ion source currently employed at the Los Alamos Neutron Science Center (LANSCE) is based on cesium enhanced surface production of H(-) ion beams in a filament-driven discharge. In this kind of an ion source the extracted H(-) beam current is limited by the achievable plasma density which depends primarily on the electron emission current from the filaments. The emission current can be increased by increasing the filament temperature but, unfortunately, this leads not only to shorter filament lifetime but also to an increase in metal evaporation from the filament, which deposits on the H(-) converter surface and degrades its performance. Therefore, we have started an ion source development project focused on replacing these thermionic cathodes (filaments) of the converter source by a helicon plasma generator capable of producing high-density hydrogen plasmas with low electron energy. In our studies which have so far shown that the plasma density of the surface conversion source can be increased significantly by exciting a helicon wave in the plasma, and we expect to improve the performance of the surface converter H(-) ion source in terms of beam brightness and time between services. The design of this new source and preliminary results are presented, along with a discussion of physical processes relevant for H(-) ion beam production with this novel design. Ultimately, we perceive this approach as an interim step towards our long-term goal, combining a helicon plasma generator with an SNS-type main discharge chamber, which will allow us to individually optimize the plasma properties of the plasma cathode (helicon) and H(-) production (main discharge) in order to further improve the brightness of extracted H(-) ion beams.

Effect of thermionic cathode heating current self-magnetic field on gaseous plasma generator characteristics

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lopatin, I. V., E-mail: lopatin@opee.hcei.tsc.ru; Akhmadeev, Yu. H.; Koval, N. N.

2015-10-15

The performance capabilities of the PINK, a plasma generator with a thermionic cathode mounted in the cavity of a hollow cathode, depending for its operation on a non-self-sustained low-pressure gas discharge have been investigated. It has been shown that when a single-filament tungsten cathode 2 mm in diameter is used and the peak filament current is equal to or higher than 100 A, the self-magnetic field of the filament current significantly affects the discharge current and voltage waveforms. This effect is due to changes in the time and space distributions of the emission current density from the hot cathode. Whenmore » the electron mean free path is close to the characteristic dimensions of the thermionic cathode, the synthesized plasma density distribution is nonuniform and the cathode is etched nonuniformly. The cathode lifetime in this case is 8–12 h. Using a cathode consisting of several parallel-connected tungsten filaments ∼0.8 mm in diameter moderates the effect of the self-magnetic field of the filament current and nearly doubles the cathode lifetime. The use of this type of cathode together with a discharge igniting electrode reduces the minimum operating pressure in the plasma generator to about one third of that required for the generator operation with a single-filament cathode (to 0.04 Pa)« less

Design and Preliminary Performance Testing of Electronegative Gas Plasma Thruster

NASA Technical Reports Server (NTRS)

Liu, Thomas M.; Schloeder, Natalie R.; Walker, Mitchell L. R.; Polzin, Kurt A.; Dankanich, John W.; Aanesland, Ane

2014-01-01

In classical gridded electrostatic ion thrusters, positively charged ions are generated from a plasma discharge of noble gas propellant and accelerated to provide thrust. To maintain overall charge balance on the propulsion system, a separate electron source is required to neutralize the ion beam as it exits the thruster. However, if high-electronegativity propellant gases (e.g., sulfur hexafluoride) are instead used, a plasma discharge can result consisting of both positively and negatively charged ions. Extracting such electronegative plasma species for thrust generation (e.g., with time-varying, bipolar ion optics) would eliminate the need for a separate neutralizer cathode subsystem. In addition for thrusters utilizing a RF plasma discharge, further simplification of the ion thruster power system may be possible by also using the RF power supply to bias the ion optics. Recently, the PEGASES (Plasma propulsion with Electronegative gases) thruster prototype successfully demonstrated proof-of-concept operations in alternatively accelerating positively and negatively charged ions from a RF discharge of a mixture of argon and sulfur hexafluoride.i In collaboration with NASA Marshall Space Flight Center (MSFC), the Georgia Institute of Technology High-Power Electric Propulsion Laboratory (HPEPL) is applying the lessons learned from PEGASES design and testing to develop a new thruster prototype. This prototype will incorporate design improvements and undergo gridless operational testing and diagnostics checkout at HPEPL in April 2014. Performance mapping with ion optics will be conducted at NASA MSFC starting in May 2014. The proposed paper discusses the design and preliminary performance testing of this electronegative gas plasma thruster prototype.

Propagation of atmospheric pressure helium plasma jet into ambient air at laminar gas flow

NASA Astrophysics Data System (ADS)

Pinchuk, M.; Stepanova, O.; Kurakina, N.; Spodobin, V.

2017-05-01

The formation of an atmospheric pressure plasma jet (APPJ) in a gas flow passing through the discharge gap depends on both gas-dynamic properties and electrophysical parameters of the plasma jet generator. The paper presents the results of experimental and numerical study of the propagation of the APPJ in a laminar flow of helium. A dielectric-barrier discharge (DBD) generated inside a quartz tube equipped with a coaxial electrode system, which provided gas passing through it, served as a plasma source. The transition of the laminar regime of gas flow into turbulent one was controlled by the photography of a formed plasma jet. The corresponding gas outlet velocity and Reynolds numbers were revealed experimentally and were used to simulate gas dynamics with OpenFOAM software. The data of the numerical simulation suggest that the length of plasma jet at the unvarying electrophysical parameters of DBD strongly depends on the mole fraction of ambient air in a helium flow, which is established along the direction of gas flow.

Pulsed Electron Source with Grid Plasma Cathode and Longitudinal Magnetic Field for Modification of Material and Product Surfaces

NASA Astrophysics Data System (ADS)

Devyatkov, V. N.; Koval, N. N.

2018-01-01

The description and the main characteristics of the pulsed electron source "SOLO" developed on the basis of the plasma cathode with grid stabilization of the emission plasma boundary are presented. The emission plasma is generated by a low-pressure arc discharge, and that allows to form the dense low-energy electron beam with a wide range of independently adjustable parameters of beam current pulses (pulse duration of 20-250 μs, pulse repetition rate of 1-10 s-1, amplitude of beam current pulses of 20-300 A, and energy of beam electrons of 5-25 keV). The special features of generation of emission plasma by constricted low-pressure arc discharge in the grid plasma cathode partially dipped into a non-uniform magnetic field and of formation and transportation of the electron beam in a longitudinal magnetic field are considered. The application area of the electron source and technologies realized with its help are specified.

Generation of X-rays and neutrons with a RF-discharge

NASA Technical Reports Server (NTRS)

Schneider, R. T.

1982-01-01

An experimental study concerning disk shaped plasma structures was performed. Such disk-shaped structures can be obtained using an rf discharge in hydrogen. The applied frequency was 1-2 Mhz. In case of operation in deuterium it was found that the discharge emits neutrons and X-rays, although the applied voltage is only 2 kV. This phenomenon was explained by assuming formation of plasma cavitons which are surrounded by high electric fields. The condition for formation of these cavitons is that the applied rf frequency is equal to the plasma frequency. The ions trapped in these resonance structures acquire sufficient energy that they can undergo fusion reactions with the ions in the surrounding gas.

Discharge pulse phenomenology

NASA Technical Reports Server (NTRS)

Frederickson, A. R.

1985-01-01

A model was developed which places radiation induced discharge pulse results into a unified conceptual framework. Only two phenomena are required to interpret all space and laboratory results: (1) radiation produces large electrostatic fields inside insulators via the trapping of a net space charge density; and (2) the electrostatic fields initiate discharge streamer plasmas similar to those investigated in high voltage electrical insulation materials; these streamer plasmas generate the pulsing phenomena. The apparent variability and diversity of results seen is an inherent feature of the plasma streamer mechanism acting in the electric fields which is created by irradiation of the dielectrics. The implications of the model are extensive and lead to constraints over what can be done about spacecraft pulsing.

Electromagnetic radiation generated by arcing in low density plasma

NASA Technical Reports Server (NTRS)

Vayner, Boris V.; Ferguson, Dale C.; Snyder, David B.; Doreswamy, C. V.

1996-01-01

An unavoidable step in the process of space exploration is to use high-power, very large spacecraft launched into Earth orbit. Obviously, the spacecraft will need powerful energy sources. Previous experience has shown that electrical discharges occur on the surfaces of a high-voltage array, and these discharges (arcs) are undesirable in many respects. Moreover, any high voltage conductor will interact with the surrounding plasma, and that interaction may result in electrical discharges between the conductor and plasma (or between two conductors with different potentials, for example, during docking and extravehicular activity). One very important aspect is the generation of electromagnetic radiation by arcing. To prevent the negative influence of electromagnetic noise on the operation of spacecraft systems, it seems necessary to determine the spectra and absolute levels of the radiation, and to determine limitations on the solar array bias voltage that depend on the parameters of LEO plasma and the technical requirements of the spacecraft equipment. This report describes the results of an experimental study and computer simulation of the electromagnetic radiation generated by arcing on spacecraft surfaces. A large set of high quality data was obtained during the Solar Array Module Plasma Interaction Experiment (SAMPIE, flight STS-62) and ground test. These data include the amplitudes of current, pulse forms, duration of each arc, and spectra of plasma waves. A theoretical explanation of the observed features is presented in this report too. The elaborated model allows us to determine the parameters of the electromagnetic noise for different frequency ranges, distances from the arcing site, and distinct kinds of plasma waves.

Kinetics of charged particles in a high-voltage gas discharge in a nonuniform electrostatic field

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kolpakov, V. A., E-mail: kolpakov683@gmail.com; Krichevskii, S. V.; Markushin, M. A.

A high-voltage gas discharge is of interest as a possible means of generating directed flows of low-temperature plasma in the off-electrode space distinguished by its original features [1–4]. We propose a model for calculating the trajectories of charges particles in a high-voltage gas discharge in nitrogen at a pressure of 0.15 Torr existing in a nonuniform electrostatic field and the strength of this field. Based on the results of our calculations, we supplement and refine the extensive experimental data concerning the investigation of such a discharge published in [1, 2, 5–8]; good agreement between the theory and experiment has beenmore » achieved. The discharge burning is initiated and maintained through bulk electron-impact ionization and ion–electron emission. We have determined the sizes of the cathode surface regions responsible for these processes, including the sizes of the axial zone involved in the discharge generation. The main effect determining the kinetics of charged particles consists in a sharp decrease in the strength of the field under consideration outside the interelectrode space, which allows a free motion of charges with specific energies and trajectories to be generated in it. The simulation results confirm that complex electrode systems that allow directed plasma flows to be generated at a discharge current of hundreds or thousands of milliamperes and a voltage on the electrodes of 0.3–1 kV can be implemented in practice [3, 9, 10].« less

Cleaning of inner vacuum surfaces in the Uragan-3M facility by radio-frequency discharges

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lozin, A. V., E-mail: alexlozin@meta.ua; Moiseenko, V. E.; Grigor’eva, L. I.

2013-08-15

A method for cleaning vacuum surfaces by a low-temperature (T{sub e} ∼ 10 eV) relatively dense (n{sub e} ≈ 10{sup 12} cm{sup −3}) plasma of an RF discharge was developed and successfully applied at the Uragan-3M torsatron. The convenience of the method is that it can be implemented with the same antenna system and RF generators that are used to produce and heat the plasma in the operating mode and does not require retuning the frequencies of the antennas and RF generators. The RF discharge has a high efficiency from the standpoint of cleaning vacuum surfaces. After performing a seriesmore » of cleanings by the low-temperature RF discharge plasma (about 20000 pulses), (i) the intensity of the CIII impurity line was substantially reduced, (ii) a quasi-steady operating mode with a duration of up to 50 ms, a plasma density of n{sub e} ≈ 10{sup 12} cm{sup −3}, and an electron temperature of up to T{sub e} ∼ 1 keV was achieved, and (iii) mass spectrometric analysis of the residual gas in the chamber indicated a significant reduction in the impurity content.« less

Ionization of Xenon to the Nickel-Like Stage and Beyond in Micro-Capillary Plasma Columns Heated by Ultrafast Current Pulses

NASA Astrophysics Data System (ADS)

Avaria, G.; Grisham, M.; Li, J.; Tomasel, F. G.; Shlyapstsev, V. N.; Busquet, M.; Woolston, M.; Rocca, J. J.

Homogeneous plasma columns with ionization levels typical of MA discharges were created by rapidly heating gas-filled 520 µm diameter channels with ns rise-time current pulses of unusually low amplitude, 40 kA. These conditions allow the generation of high aspect ratio (eg. > 300:1) plasma columns with very high degrees of ionization (e.g. Ni-like Xenon) of interest for soft x-ray lasers below λ = 10 nm. Spectra and simulations of plasmas generated in 520 µm diameter alumina capillaries driven by 35-40 kA current pulses with 4 ns rise time were obtained for discharges in Xenon and Neon discharges. The first shows the presence of lines corresponding to ionization stages up to Fe-like Xe. The latter show that Al impurities from the walls are ionized to the H-like and He-like stages. He-like Al spectra containing the resonance line significantly broaden by opacity, the intercombination line, and Li-like satellites are analyzed. For Xenon discharges, the spectral lines from the Ni-like transitions the 3d94d (3/2, 3/2)J = 0 to the 3d94p(5/2, 3/2)J = 1 and to 3d94p(3/2, 1/2)J = 1 are observed.

Arcing in LEO: Does the Whole Array Discharge?

NASA Technical Reports Server (NTRS)

Ferguson, Dale C.; Vayner, Boris V.; Galofaro, Joel T.; Hillard, G. Barry

2005-01-01

The conventional wisdom about solar array arcing in LEO is that only the parts of the solar array that are swept over by the arc-generated plasma front are discharged in the initial arc. This limits the amount of energy that can be discharged. Recent work done at the NASA Glenn Research Center has shown that this idea is mistaken. In fact, the capacitance of the entire solar array may be discharged, which for large arrays leads to very large and possibly debilitating arcs, even if no sustained arc occurs. We present the laboratory work that conclusively demonstrates this fact by using a grounded plate that prevents the arc-plasma front from reaching certain array strings. Finally, we discuss the dependence of arc strength and arc pulse width on the capacitance that is discharged, and provide a physical mechanism for discharge of the entire array, even when parts of the array are not accessible to the arc-plasma front. Mitigation techniques are also presented.

Comparison of runaway electron generation parameters in small, medium-sized and large tokamaks—A survey of experiments in COMPASS, TCV, ASDEX-Upgrade and JET

NASA Astrophysics Data System (ADS)

Plyusnin, V. V.; Reux, C.; Kiptily, V. G.; Pautasso, G.; Decker, J.; Papp, G.; Kallenbach, A.; Weinzettl, V.; Mlynar, J.; Coda, S.; Riccardo, V.; Lomas, P.; Jachmich, S.; Shevelev, A. E.; Alper, B.; Khilkevitch, E.; Martin, Y.; Dux, R.; Fuchs, C.; Duval, B.; Brix, M.; Tardini, G.; Maraschek, M.; Treutterer, W.; Giannone, L.; Mlynek, A.; Ficker, O.; Martin, P.; Gerasimov, S.; Potzel, S.; Paprok, R.; McCarthy, P. J.; Imrisek, M.; Boboc, A.; Lackner, K.; Fernandes, A.; Havlicek, J.; Giacomelli, L.; Vlainic, M.; Nocente, M.; Kruezi, U.; COMPASS Team; TCV Team; ASDEX-Upgrade Team; EUROFusion MST1 Team; contributors, JET

2018-01-01

This paper presents a survey of the experiments on runaway electrons (RE) carried out recently in frames of EUROFusion Consortium in different tokamaks: COMPASS, ASDEX-Upgrade, TCV and JET. Massive gas injection (MGI) has been used in different scenarios for RE generation in small and medium-sized tokamaks to elaborate the most efficient and reliable ones for future RE experiments. New data on RE generated at disruptions in COMPASS and ASDEX-Upgrade was collected and added to the JET database. Different accessible parameters of disruptions, such as current quench rate, conversion rate of plasma current into runaways, etc have been analysed for each tokamak and compared to JET data. It was shown, that tokamaks with larger geometrical sizes provide the wider limits for spatial and temporal variation of plasma parameters during disruptions, thus extending the parameter space for RE generation. The second part of experiments was dedicated to study of RE generation in stationary discharges in COMPASS, TCV and JET. Injection of Ne/Ar have been used to mock-up the JET MGI runaway suppression experiments. Secondary RE avalanching was identified and quantified for the first time in the TCV tokamak in RE generating discharges after massive Ne injection. Simulations of the primary RE generation and secondary avalanching dynamics in stationary discharges has demonstrated that RE current fraction created via avalanching could achieve up to 70-75% of the total plasma current in TCV. Relaxations which are reminiscent the phenomena associated to the kinetic instability driven by RE have been detected in RE discharges in TCV. Macroscopic parameters of RE dominating discharges in TCV before and after onset of the instability fit well to the empirical instability criterion, which was established in the early tokamaks and examined by results of recent numerical simulations.

Note: Design and investigation of a multichannel plasma-jet triggered gas switch.

PubMed

Tie, Weihao; Liu, Xuandong; Zhang, Qiaogen; Liu, Shanhong

2014-07-01

We described the fabrication and testing of a multichannel plasma-jet triggered gas switch (MPJTGS). A novel six-channel annular micro-plasma-gun was embedded in the trigger electrode to generate multichannel plasma jets as a nanosecond trigger pulse arrived. The gas breakdown in multiple sites of the spark gap was induced and fixed around jet orifices by the plasma jets. We tested the multichannel discharge characteristics of the MPJTGS in two working modes with charge voltage of 50 kV, trigger voltage of +40 kV (25 ns rise time), and trigger energy of 240 J, 32 J, and 2 J, respectively, at different working coefficients. Results show that the average number of discharge channels increased as the trigger energy increased, and decreased as the working coefficient decreased. At a working coefficient of 87.1% and trigger energy of 240 J, the average number of discharge channels in Mode II could reach 4.1.

Laser sustained discharge nozzle apparatus for the production of an intense beam of high kinetic energy atomic species

DOEpatents

Cross, Jon B.; Cremers, David A.

1988-01-01

Laser sustained discharge apparatus for the production of intense beams of high kinetic energy atomic species. A portion of the plasma resulting from a laser sustained continuous optical discharge which generates energetic atomic species from a gaseous source thereof is expanded through a nozzle into a region of low pressure. The expanded plasma contains a significant concentration of the high kinetic energy atomic species which may be used to investigate the interaction of surfaces therewith. In particular, O-atoms having velocities in excess of 3.5 km/s can be generated for the purpose of studying their interaction with materials in order to develop protective materials for spacecraft which are exposed to such energetic O-atoms during operation in low earth orbit.

Laser sustained discharge nozzle apparatus for the production of an intense beam of high kinetic energy atomic species

DOEpatents

Cross, J.B.; Cremers, D.A.

1986-01-10

Laser sustained discharge apparatus for the production of intense beams of high kinetic energy atomic species is described. A portion of the plasma resulting from a laser sustained continuous optical discharge which generates energetic atomic species from a gaseous source thereof is expanded through a nozzle into a region of low pressure. The expanded plasma contains a significant concentration of the high kinetic energy atomic species which may be used to investigate the interaction of surfaces therewith. In particular, O-atoms having velocities in excess of 3.5 km/s can be generated for the purpose of studying their interaction with materials in order to develop protective materials for spacecraft which are exposed to such energetic O-atoms during operation in low earth orbit.

Effects of pulse frequency of input power on the physical and chemical properties of pulsed streamer discharge plasmas in water

NASA Astrophysics Data System (ADS)

Ruma; Lukes, P.; Aoki, N.; Spetlikova, E.; Hosseini, S. H. R.; Sakugawa, T.; Akiyama, H.

2013-03-01

A repetitive pulsed-power modulator, which employs a magnetic pulse compression circuit with a high-speed thyristor switch, was used to study the effects of the pulse repetition rate of input power on the physical and chemical properties of pulsed discharges in water. Positive high-voltage pulses of 20 kV with repetition rates of up to 1 kHz were used to generate a discharge in water using the point-to-plane electrode geometry. By varying the pulse repetition rate, two distinct modes of the discharge plasma were formed in water. The first mode was characterized by the formation of a corona-like discharge propagating through water in the form of streamer channels. The second mode was formed typically above 500 Hz, when the formation of streamer channels in water was suppressed and all plasmas occurred inside a spheroidal aggregate of very fine gas bubbles surrounding the tip of the high-voltage electrode. The production of hydrogen peroxide, degradation of organic dye Acid Orange 7 (AO7) and inactivation of bacteria Escherichia coli by the discharge in water were studied under different discharge plasma modes in dependence on the pulse repetition rate of input power. The efficiency of both chemical and biocidal processes induced by the plasma in water decreased significantly with pulse repetition rates above 500 Hz.

Measurements and Simulations of Surface Dielectric Barrier Discharges Used as Plasma Actuators

NASA Technical Reports Server (NTRS)

Hoskinson, Alan R.

2012-01-01

This report is a Ph.D. dissertation performed under NRA cooperative agreement and submitted as part of the final report. Asymmetric surface dielectric barrier discharges (DBDs) have shown promise for use as aerodynamic actuators for active flow control. In this project we studied DBD actuators experimentally and numerically. Our DBDs used a symmetric triangular high voltage waveform to generate plasma in atmospheric pressure air. Time-averaged measurements indicated that the induced force of a single barrier actuator design (one electrode insulated from the plasma) can be increased exponentially above the results of previous studies by decreasing both the length and thickness of the electrode exposed to the plasma. This increased force may allow these devices to control flow separation in a wider range of flow environments. Experiments using an intensified digital camera to examine the plasma on time scales of a few nanoseconds showed that, in addition to the previously-observed filamentary and jet-like plasma structures, discharges with very thin exposed electrodes exhibited a weak but constant plasma immediately adjacent to those electrodes. In double-barrier actuators (both electrodes insulated), decreasing the diameter of the narrower electrode lead to increasing forces, and recorded images showed the simultaneous existence of both filamentary and jet-like plasma structures. The development and application of a time-dependent, two-dimensional computational fluid plasma model has aided in understanding the detailed physics of surface DBDs at all-time scales. For simulated single-barrier discharges, the model qualitatively reproduced the filamentary and jet-like micro-discharge structures. The model was somewhat successful in reproducing the observed characteristics of double-barrier actuators. For both actuator geometries, the model indicated that the majority of the forces induced on the neutral gas occur in between micro-discharges as the plasmas decay.

Generation of tunable plasma photonic crystals in meshed dielectric barrier discharge

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang, Yongjie; Dong, Lifang, E-mail: donglfhbu@163.com; Liu, Weibo

2014-07-15

Tunable superlattice plasma photonic crystals are obtained in a meshed dielectric barrier discharge. These plasma photonic crystals are composed of thin artificial lattices and thick self-organized lattices, and can be tuned easily by adjusting the applied voltage. A plasma photonic crystal with self-organized hexagonal lattice coupled to artificial square lattice is first realized. The dispersion relations of the square sublattices with different radii, which are recorded by an intensified charge-coupled device camera, are calculated. The results show that the thick square sublattice has the higher band edge frequencies and wider band widths. Band gaps of superlattice plasma photonic crystals aremore » actually temporal integrations of those of transient sublattices.« less

Plasma-enhanced mixing and flameholding in supersonic flow

PubMed Central

Firsov, Alexander; Savelkin, Konstantin V.; Yarantsev, Dmitry A.; Leonov, Sergey B.

2015-01-01

The results of experimental study of plasma-based mixing, ignition and flameholding in a supersonic model combustor are presented in the paper. The model combustor has a length of 600 mm and cross section of 72 mm width and 60 mm height. The fuel is directly injected into supersonic airflow (Mach number M=2, static pressure Pst=160–250 Torr) through wall orifices. Two series of tests are focused on flameholding and mixing correspondingly. In the first series, the near-surface quasi-DC electrical discharge is generated by flush-mounted electrodes at electrical power deposition of Wpl=3–24 kW. The scope includes parametric study of ignition and flame front dynamics, and comparison of three schemes of plasma generation: the first and the second layouts examine the location of plasma generators upstream and downstream from the fuel injectors. The third pattern follows a novel approach of combined mixing/ignition technique, where the electrical discharge distributes along the fuel jet. The last pattern demonstrates a significant advantage in terms of flameholding limit. In the second series of tests, a long discharge of submicrosecond duration is generated across the flow and along the fuel jet. A gasdynamic instability of thermal cavity developed after a deposition of high-power density in a thin plasma filament promotes the air–fuel mixing. The technique studied in this work has weighty potential for high-speed combustion applications, including cold start/restart of scramjet engines and support of transition regime in dual-mode scramjet and at off-design operation. PMID:26170434

Dependence of electron peak current on hollow cathode dimensions and seed electron energy in a pseudospark discharge

NASA Astrophysics Data System (ADS)

Cetiner, S. O.; Stoltz, P.; Messmer, P.; Cambier, J.-L.

2008-01-01

The prebreakdown and breakdown phases of a pseudospark discharge are investigated using the two-dimensional kinetic plasma simulation code OOPIC™ PRO. Trends in the peak electron current at the anode are presented as function of the hollow cathode dimensions and mean seed injection velocities at the cavity back wall. The plasma generation process by ionizing collisions is examined, showing the effect on supplying the electrons that determine the density of the beam. The mean seed velocities used here are varied between the velocity corresponding to the energy of peak ionization cross section, 15 times this value and no mean velocity (i.e., electrons injected with a temperature of 2.5eV). The reliance of the discharge characteristics on the penetrating electric field is shown to decrease as the mean seed injection velocity increases because of its ability to generate a surplus plasma independent of the virtual anode. As a result, the peak current increases with the hollow cathode dimensions for the largest average injection velocity, while for the smallest value it increases with the area of penetration of the electric field in the hollow cathode interior. Additionally, for a given geometry an increase in the peak current with the surplus plasma generated is observed. For the largest seed injection velocity used a dependence of the magnitude of the peak current on the ratio of the hole thickness and hollow cathode depth to the hole height is demonstrated. This means similar trends of the peak current are generated when the geometry is resized. Although the present study uses argon only, the variation in the discharge dependencies with the seed injection energy relative to the ionization threshold is expected to apply independently of the gas type. Secondary electrons due to electron and ion impact are shown to be important only for the largest impact areas and discharge development times of the study.

Hydrogen and Ethene Plasma Assisted Ignition by NS discharge at Elevated Temperatures

NASA Astrophysics Data System (ADS)

Starikovskiy, Andrey

2015-09-01

The kinetics of ignition in lean H2:O2:Ar and C2H4:O2:Ar mixtures has been studied experimentally and numerically after a high-voltage nanosecond discharge. The ignition delay time behind a reflected shock wave was measured with and without the discharge. It was shown that the initiation of the discharge with a specific deposited energy of 10 - 30 mJ/cm3 leads to an order of magnitude decrease in the ignition delay time. Discharge processes and following chain chemical reactions with energy release were simulated. The generation of atoms, radicals and excited and charged particles was numerically simulated using the measured time - resolved discharge current and electric field in the discharge phase. The calculated densities of the active particles were used as input data to simulate plasma-assisted ignition. Good agreement was obtained between the calculated ignition delay times and the experimental data. It follows from the analysis of the calculated results that the main mechanism of the effect of gas discharge on the ignition of hydrocarbons is the electron impact dissociation of O2 molecules in the discharge phase. Detailed kinetic mechanism for plasma assisted ignition of hydrogen and ethene is elaborated and verified.

RF power absorption by plasma of low pressure low power inductive discharge located in the external magnetic field

NASA Astrophysics Data System (ADS)

Kralkina, E. A.; Rukhadze, A. A.; Nekliudova, P. A.; Pavlov, V. B.; Petrov, A. K.; Vavilin, K. V.

2018-03-01

Present paper is aimed to reveal experimentally and theoretically the influence of magnetic field strength, antenna shape, pressure, operating frequency and geometrical size of plasma sources on the ability of plasma to absorb the RF power characterized by the equivalent plasma resistance for the case of low pressure RF inductive discharge located in the external magnetic field. The distinguishing feature of the present paper is the consideration of the antennas that generate not only current but charge on the external surface of plasma sources. It is shown that in the limited plasma source two linked waves can be excited. In case of antennas generating only azimuthal current the waves can be attributed as helicon and TG waves. In the case of an antenna with the longitudinal current there is a surface charge on the side surface of the plasma source, which gives rise to a significant increase of the longitudinal and radial components of the RF electric field as compared with the case of the azimuthal antenna current.

Methane chemistry involved in a low-pressure electron cyclotron wave resonant plasma discharge

NASA Astrophysics Data System (ADS)

Morrison, N. A.; William, C.; Milne, W. I.

2003-12-01

Radio frequency (rf) generated methane plasmas are commonly employed in the deposition of hydrogenated amorphous carbon (a-C:H) thin films. However, very little is known about the rf discharge chemistry and how it relates to the deposition process. Consequently, we have characterized a low-pressure methane plasma and compared the results with those obtained theoretically by considering the steady-state kinetics of the chemical processes present in a low-pressure plasma reactor, in order to elucidate the dominant reaction channels responsible for the generation of the active precursors required for film growth. Mass spectrometry measurements of the gas phase indicated little variation in the plasma chemistry with increasing electron temperature. This was later attributed to the partial saturation of the electron-impact dissociation and ionization rate constants at electron temperatures in excess of ˜4 eV. The ion densities in the plasma were also found to be strongly dependent upon the parent neutral concentration in the gas phase, indicating that direct electron-impact reactions exerted greater influence on the plasma chemistry than secondary ion-neutral reactions.

Ion extraction from a saddle antenna RF surface plasma source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dudnikov, V., E-mail: vadim@muonsinc.com; Johnson, R. P.; Han, B.

Existing RF Surface Plasma Sources (SPS) for accelerators have specific efficiencies for H{sup +} and H{sup −} ion generation around 3 to 5 mA/cm{sup 2} per kW, where about 50 kW of RF power is typically needed for 50 mA beam current production. The Saddle Antenna (SA) SPS described here was developed to improve H{sup −} ion production efficiency and SPS reliability and availability. At low RF power, the efficiency of positive ion generation in the plasma has been improved to 200 mA/cm{sup 2} per kW of RF power at 13.56 MHz. Initial cesiation of the SPS was performed bymore » heating cesium chromate cartridges by discharge as was done in the very first versions of the SPS. A small oven to decompose cesium compounds and alloys was developed and tested. After cesiation, the current of negative ions to the collector was increased from 1 mA to 10 mA with RF power ∼1.5 kW in the plasma (6 mm diameter emission aperture) and up to 30 mA with ∼4 kW RF power in the plasma and 250 Gauss longitudinal magnetic field. The ratio of electron current to negative ion current was improved from 30 to 2. Stable generation of H{sup −} beam without intensity degradation was demonstrated in the AlN discharge chamber for a long time at high discharge power in an RF SPS with an external antenna. Continuous wave (CW) operation of the SA SPS has been tested on the small test stand. The general design of the CW SA SPS is based on the pulsed version. Some modifications were made to improve the cooling and cesiation stability. The extracted collector current can be increased significantly by optimizing the longitudinal magnetic field in the discharge chamber. CW operation with negative ion extraction was tested with RF power up to 1.8 kW from the generator (∼1.2 kW in the plasma) with production up to Ic=7 mA. Long term operation was tested with 1.2 kW from the RF generator (∼0.8 kW in the plasma) with production of Ic=5 mA, Iex ∼15 mA (Uex=8 kV, Uc=14 kV)« less

Ion extraction from a saddle antenna RF surface plasma source

NASA Astrophysics Data System (ADS)

Dudnikov, V.; Johnson, R. P.; Han, B.; Murray, S.; Pennisi, T.; Piller, C.; Santana, M.; Stockli, M.; Welton, R.; Breitschopf, J.; Dudnikova, G.

2015-04-01

Existing RF Surface Plasma Sources (SPS) for accelerators have specific efficiencies for H+ and H- ion generation around 3 to 5 mA/cm2 per kW, where about 50 kW of RF power is typically needed for 50 mA beam current production. The Saddle Antenna (SA) SPS described here was developed to improve H- ion production efficiency and SPS reliability and availability. At low RF power, the efficiency of positive ion generation in the plasma has been improved to 200 mA/cm2 per kW of RF power at 13.56 MHz. Initial cesiation of the SPS was performed by heating cesium chromate cartridges by discharge as was done in the very first versions of the SPS. A small oven to decompose cesium compounds and alloys was developed and tested. After cesiation, the current of negative ions to the collector was increased from 1 mA to 10 mA with RF power ˜1.5 kW in the plasma (6 mm diameter emission aperture) and up to 30 mA with ˜4 kW RF power in the plasma and 250 Gauss longitudinal magnetic field. The ratio of electron current to negative ion current was improved from 30 to 2. Stable generation of H- beam without intensity degradation was demonstrated in the AlN discharge chamber for a long time at high discharge power in an RF SPS with an external antenna. Continuous wave (CW) operation of the SA SPS has been tested on the small test stand. The general design of the CW SA SPS is based on the pulsed version. Some modifications were made to improve the cooling and cesiation stability. The extracted collector current can be increased significantly by optimizing the longitudinal magnetic field in the discharge chamber. CW operation with negative ion extraction was tested with RF power up to 1.8 kW from the generator (˜1.2 kW in the plasma) with production up to Ic=7 mA. Long term operation was tested with 1.2 kW from the RF generator (˜0.8 kW in the plasma) with production of Ic=5 mA, Iex ˜15 mA (Uex=8 kV, Uc=14 kV).

High frequency plasma generator for ion thrusters

NASA Technical Reports Server (NTRS)

Goede, H.; Divergilio, W. F.; Fosnight, V. V.; Komatsu, G.

1984-01-01

The results of a program to experimentally develop two new types of plasma generators for 30 cm electrostatic argon ion thrusters are presented. The two plasma generating methods selected for this study were by radio frequency induction (RFI), operating at an input power frequency of 1 MHz, and by electron cyclotron heating (ECH) at an operating frequency of 5.0 GHz. Both of these generators utilize multiline cusp permanent magnet configurations for plasma confinement and beam profile optimization. The program goals were to develop a plasma generator possessing the characteristics of high electrical efficiency (low eV/ion) and simplicity of operation while maintaining the reliability and durability of the conventional hollow cathode plasma sources. The RFI plasma generator has achieved minimum discharge losses of 120 eV/ion while the ECH generator has obtained 145 eV/ion, assuming a 90% ion optical transparency of the electrostatic acceleration system. Details of experimental tests with a variety of magnet configurations are presented.

[Spectral investigation of atmospheric pressure plasma column].

PubMed

Li, Xue-Chen; Chang, Yuan-Yuan; Xu, Long-Fei

2012-07-01

Atmospheric pressure plasma column has many important applications in plasma stealth for aircraft. In the present paper, a plasma column with a length of 65 cm was generated in argon at atmospheric pressure by using dielectric barrier discharge device with water electrodes in coaxial configurations. The discharge mechanism of the plasma column was studied by optical method and the result indicates that a moving layer of light emission propagates in the upstream region. The propagation velocity of the plasma bullet is about 0.6 x 10(5) m x s(-1) through optical measurement. Spectral intensity ratios as functions of the applied voltage and driving frequency were also investigated by spectroscopic method. The variation in spectral intensity ratio implies a change in the averaged electron energy. Results show that the averaged electron energy increases with the increase in the applied voltage and the driving frequency. These results have significant values for industrial applications of the atmospheric pressure discharge and have extensive application potentials in stealth for military aircraft.

Characterization of novel pin-hole based plasma source for generation of discharge in liquids supplied by DC non-pulsing voltage

NASA Astrophysics Data System (ADS)

Krčma, F.; Kozáková, Z.; Mazánková, V.; Horák, J.; Dostál, L.; Obradović, B.; Nikiforov, A.; Belmonte, T.

2018-06-01

A recently presented novel plasma source generating discharge in liquids based on the pin-hole discharge configuration is characterized in detail. The system is supplied by DC non-pulsing high voltage of both polarities in NaCl water solutions at a conductivity range of 100–15 000 μS/cm. The discharge itself shows self-pulsing operation. The discharge ignition is observed in micro bubbles by transient discharge followed by a glow discharge in positive polarity at lower conductivities propagating inside the bubbles. At high conductivities, the glow regime is particularly replaced by a more energetic sequence of transient discharges followed by a shorter glow mode operation. The transient regime probability and its intensity are higher in the negative discharge polarity. The transient discharge produces acoustic waves and shock waves, which are observed at the moment of the bubble cavitation. The average gas temperature of 700–1500 K was calculated from the lowest OH (A-X) 0-0 band transitions. The average electron concentrations of 1020–1023 m‑3 were calculated from H α and H β line profiles. Finally, the production of a chemically active species is determined by hydrogen peroxide energy yields related to the energy consumption of the whole interelectrode system. All these quantities are dependent on the solution conductivity, the discharge polarity, and the applied power.

Modification of W surfaces by exposure to hollow cathode plasmas

NASA Astrophysics Data System (ADS)

Stancu, C.; Stokker-Cheregi, F.; Moldovan, A.; Dinescu, M.; Grisolia, C.; Dinescu, G.

2017-10-01

In this work, we assess the surface modifications induced on W samples following exposure to He and He/H2 radiofrequency plasmas in hollow cathode discharge configuration. Our study addresses issues that relate to the use of W in next-generation fusion reactors and, therefore, the investigation of W surface degradation following exposure and heating by plasmas to temperatures above 1000 °C is of practical importance. For these experiments, we used commercially available tungsten samples having areas of 30 × 15 mm and 0.1 mm thickness. The hollow cathode plasma was produced using a radiofrequency (RF) generator (13.56 MHz) between parallel plate electrodes. The W samples were mounted as one of the electrodes. The He and He/H2 plasma discharges had a combined effect of heating and bombardment of the W surfaces. The surface modifications were studied for discharge powers between 200 and 300 W, which resulted in the heating of the samples to temperatures between 950 and 1230 °C, respectively. The samples were weighed prior and after plasma exposure, and loss of mass was measured following plasma exposure times up to 90 min. The analysis of changes in surface morphology was carried out by optical microscopy, scanning electron microscopy and atomic force microscopy. Additionally, optical emission spectra of the respective plasmas were recorded from the region localized inside the hollow cathode gap. We discuss the influence of experimental parameters on the changes in surface morphology.

Pure rotational CARS thermometry studies of low-temperature oxidation kinetics in air and ethene-air nanosecond pulse discharge plasmas

NASA Astrophysics Data System (ADS)

Zuzeek, Yvette; Choi, Inchul; Uddi, Mruthunjaya; Adamovich, Igor V.; Lempert, Walter R.

2010-03-01

Pure rotational CARS thermometry is used to study low-temperature plasma assisted fuel oxidation kinetics in a repetitive nanosecond pulse discharge in ethene-air at stoichiometric and fuel lean conditions at 40 Torr pressure. Air and fuel-air mixtures are excited by a burst of high-voltage nanosecond pulses (peak voltage, 20 kV; pulse duration, ~ 25 ns) at a 40 kHz pulse repetition rate and a burst repetition rate of 10 Hz. The number of pulses in the burst is varied from a few pulses to a few hundred pulses. The results are compared with the previously developed hydrocarbon-air plasma chemistry model, modified to incorporate non-empirical scaling of the nanosecond discharge pulse energy coupled to the plasma with number density, as well as one-dimensional conduction heat transfer. Experimental time-resolved temperature, determined as a function of the number of pulses in the burst, is found to agree well with the model predictions. The results demonstrate that the heating rate in fuel-air plasmas is much faster compared with air plasmas, primarily due to energy release in exothermic reactions of fuel with O atoms generated by the plasma. It is found that the initial heating rate in fuel-air plasmas is controlled by the rate of radical (primarily O atoms) generation and is nearly independent of the equivalence ratio. At long burst durations, the heating rate in lean fuel air-mixtures is significantly reduced when all fuel is oxidized.

Energy efficiency in nanoscale synthesis using nanosecond plasmas.

PubMed

Pai, David Z; Ken Ostrikov, Kostya; Kumar, Shailesh; Lacoste, Deanna A; Levchenko, Igor; Laux, Christophe O

2013-01-01

We report a nanoscale synthesis technique using nanosecond-duration plasma discharges. Voltage pulses 12.5 kV in amplitude and 40 ns in duration were applied repetitively at 30 kHz across molybdenum electrodes in open ambient air, generating a nanosecond spark discharge that synthesized well-defined MoO₃ nanoscale architectures (i.e. flakes, dots, walls, porous networks) upon polyamide and copper substrates. No nitrides were formed. The energy cost was as low as 75 eV per atom incorporated into a nanostructure, suggesting a dramatic reduction compared to other techniques using atmospheric pressure plasmas. These findings show that highly efficient synthesis at atmospheric pressure without catalysts or external substrate heating can be achieved in a simple fashion using nanosecond discharges.

Detection and removal of impurities in nitric oxide generated from air by pulsed electrical discharge.

PubMed

Yu, Binglan; Blaesi, Aron H; Casey, Noel; Raykhtsaum, Grigory; Zazzeron, Luca; Jones, Rosemary; Morrese, Alexander; Dobrynin, Danil; Malhotra, Rajeev; Bloch, Donald B; Goldstein, Lee E; Zapol, Warren M

2016-11-30

Inhalation of nitric oxide (NO) produces selective pulmonary vasodilation without dilating the systemic circulation. However, the current NO/N 2 cylinder delivery system is cumbersome and expensive. We developed a lightweight, portable, and economical device to generate NO from air by pulsed electrical discharge. The objective of this study was to investigate and optimize the purity and safety of NO generated by this device. By using low temperature streamer discharges in the plasma generator, we produced therapeutic levels of NO with very low levels of nitrogen dioxide (NO 2 ) and ozone. Despite the low temperature, spark generation eroded the surface of the electrodes, contaminating the gas stream with metal particles. During prolonged NO generation there was gradual loss of the iridium high-voltage tip (-90 μg/day) and the platinum-nickel ground electrode (-55 μg/day). Metal particles released from the electrodes were trapped by a high-efficiency particulate air (HEPA) filter. Quadrupole mass spectroscopy measurements of effluent gas during plasma NO generation showed that a single HEPA filter removed all of the metal particles. Mice were exposed to breathing 50 parts per million of electrically generated NO in air for 28 days with only a scavenger and no HEPA filter; the mice did not develop pulmonary inflammation or structural changes and iridium and platinum particles were not detected in the lungs of these mice. In conclusion, an electric plasma generator produced therapeutic levels of NO from air; scavenging and filtration effectively eliminated metallic impurities from the effluent gas. Copyright © 2016 Elsevier Inc. All rights reserved.

Detection and Removal of Impurities in Nitric Oxide Generated from Air by Pulsed Electrical Discharge

PubMed Central

Yu, Binglan; Blaesi, Aron H.; Casey, Noel; Raykhtsaum, Grigory; Zazzeron, Luca; Jones, Rosemary; Morrese, Alexander; Dobrynin, Danil; Malhotra, Rajeev; Bloch, Donald B.; Goldstein, Lee E.; Zapol, Warren M.

2016-01-01

Inhalation of nitric oxide (NO) produces selective pulmonary vasodilation without dilating the systemic circulation. However, the current NO/N2 cylinder delivery system is cumbersome and expensive. We developed a lightweight, portable, and economical device to generate NO from air by pulsed electrical discharge. The objective of this study was to investigate and optimize the purity and safety of NO generated by this device. By using low temperature streamer discharges in the plasma generator, we produced therapeutic levels of NO with very low levels of nitrogen dioxide (NO2) and ozone. Despite the low temperature, spark generation eroded the surface of the electrodes, contaminating the gas stream with metal particles. During prolonged NO generation there was gradual loss of the iridium high-voltage tip (−90 µg/day) and the platinum-nickel ground electrode (−55 µg/day). Metal particles released from the electrodes were trapped by a high-efficiency particulate air (HEPA) filter. Quadrupole mass spectroscopy measurements of effluent gas during plasma NO generation showed that a single HEPA filter removed all of the metal particles. Mice were exposed to breathing 50 parts per million of electrically generated NO in air for 28 days with only a scavenger and no HEPA filter; the mice did not develop pulmonary inflammation or structural changes and iridium and platinum particles were not detected in the lungs of these mice. In conclusion, an electric plasma generator produced therapeutic levels of NO from air; scavenging and filtration effectively eliminated metallic impurities from the effluent gas. PMID:27592386

Discharge processes and an electrical model of atmospheric pressure plasma jets in argon

NASA Astrophysics Data System (ADS)

Fang, Zhi; Shao, Tao; Yang, Jing; Zhang, Cheng

2016-01-01

In this paper, an atmospheric pressure plasma discharge in argon was generated using a needle-to-ring electrode configuration driven by a sinusoidal excitation voltage. The electric discharge processes and discharge characteristics were investigated by inspecting the voltage-current waveforms, Lissajous curves and lighting emission images. The change in discharge mode with applied voltage amplitude was studied and characterised, and three modes of corona discharge, dielectric barrier discharge (DBD) and jet discharge were identified, which appeared in turn with increasing applied voltage and can be distinguished clearly from the measured voltage-current waveforms, light-emission images and the changing gradient of discharge power with applied voltage. Based on the experimental results and discharge mechanism analysis, an equivalent electrical model and the corresponding equivalent circuit for characterising the whole discharge processes accurately was proposed, and the three discharge stages were characterised separately. A voltage-controlled current source (VCCS) associated with a resistance and a capacitance were used to represent the DBD stage, and the plasma plume and corona discharge were modelled by a variable capacitor in series with a variable resistor. Other factors that can influence the discharge, such as lead and stray capacitance values of the circuit, were also considered in the proposed model. Contribution to the Topical Issue "Recent Breakthroughs in Microplasma Science and Technology", edited by Kurt Becker, Jose Lopez, David Staack, Klaus-Dieter Weltmann and Wei Dong Zhu.

Radio-frequency plasma transducer for use in harsh environments.

PubMed

May, Andrew; Andarawis, Emad

2007-10-01

We describe a compact transducer used to generate and modulate low-intensity radio-frequency atmospheric pressure plasma (RF-APP) for high temperature gap measurement and generation of air-coupled ultrasound. The new transducer consists of a quarter-wave transmission line where the ground return path is a coaxial solenoid winding. The RF-APP is initiated at the open end of the transmission line and stabilized by passive negative feedback between the electrical impedance of the plasma and the energy stored in the solenoid. The electrical impedance of the plasma was measured at the lower-voltage source end of the transducer, eliminating the need to measure kilovolt-level voltages near the discharge. We describe the use of a 7 MHz RF-APP prototype as a harsh-environment clearance sensor to demonstrate the suitability of plasma discharges for a common nondestructive inspection application. Clearance measurements of 0-5 mm were performed on a rotating calibration target with a measurement precision of 0.1 mm and a 20 kHz sampling rate.

Cyclic powder formation during pulsed injection of hexamethyldisiloxane in an axially asymmetric radiofrequency argon discharge

DOE Office of Scientific and Technical Information (OSTI.GOV)

Despax, B.; Makasheva, K.; CNRS, LAPLACE, F-31062 Toulouse cedex 09

2012-11-01

A new approach of periodic production of dusty plasma consisting of pulsed injection of hexamethyldisiloxane (HMDSO) in argon axially asymmetric radiofrequency (RF) discharge was investigated in this work. The range of plasma operating conditions in which this dusty plasma can exist was closely examined. The obtained results clearly show that a net periodicity in the formation/disappearance of dust particles in the plasma can be maintained on a very large scale of discharge duration. The significance of discharge axial asymmetry to the dust particles behaviour in the plasma is revealed by the development of an asymmetric in shape void shifted towardsmore » the powered RF electrode. The key role of the reactive gas and its pulsed injection on each stage of the oscillating process of formation/disappearance of dust particles is disclosed by optical and electrical measurements. It is shown that the period of dusty plasma formation/disappearance is inversely related to the HMDSO injection time. Moreover, the impact of time injection over short period (5 s) is examined. It indicates the conflicting role played by the HMDSO on the reduction of dusty plasma during the reactive gas injection and the reappearance of particles in the plasma during the time off. The electronegative behavior of the plasma in the presence of negatively charged particles seems to explain the energetic modifications in the discharge. A frequency analysis of the floating potential reveals all these cyclic processes. Particularly, in the 10-200 Hz frequency range, the presence and the evolution of dust particles in the plasma over one generation can be observed.« less

Determination of trace cadmium in rice by liquid spray dielectric barrier discharge induced plasma - chemical vapor generation coupled with atomic fluorescence spectrometry

NASA Astrophysics Data System (ADS)

Liu, Xing; Zhu, Zhenli; Bao, Zhengyu; Zheng, Hongtao; Hu, Shenghong

2018-03-01

Cadmium contamination in rice has become an increasing concern in many countries including China. A simple, cost-effective, and highly sensitive method was developed for the determination of trace cadmium in rice samples based on a new high-efficient liquid spray dielectric barrier discharge induced plasma (LSDBD) vapor generation coupled with atomic fluorescence spectrometry (AFS). The analytical procedure involves the efficient formation of Cd volatile species by LSDBD plasma induced chemical processes without the use of any reducing reagents (Na/KBH4 in conventional hydride generation). The effects of the addition of organic substances, different discharge parameters such as discharge voltage and discharge gap, as well as the foreign ion interferences were investigated. Under optimized conditions, a detection limit of 0.01 μg L- 1 and a precision of 0.8% (RSD, n = 5, 1 μg L- 1 Cd) was readily achieved. The calibration curve was linear in the range between 0.1 and 10 μg L- 1, with a correlation coefficient of R2 = 0.9995. Compared with the conventional acid-BH4- vapor generation, the proposed method not only eliminates the use of unstable and expensive reagents, but also offers high tolerance for coexisting ions, which is well suited to the direct analysis of environmental samples. The validation of the proposed method was demonstrated by the analysis of Cd in reference material of rice (GBW080684). It was also successfully applied to the determination of trace cadmium in locally collected 11 rice samples, and the obtained Cd concentrations are ranged from 7.2 to 517.7 μg kg- 1.

Plasma characteristics of argon glow discharge produced by AC power supply operating at low frequencies

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kongpiboolkid, Watcharapon; Mongkolnavin, Rattachat; Plasma Technology and Nuclear Fusion Research Unit, Chulalongkorn University, Bangkok

2015-04-24

Non-thermal properties of Argon glow discharge operating with various operating pressures were measured and presented in this work. The Argon plasma is produced by a parallel conducting electrodes coupling with a high voltage AC power supply. The power supply can generate high AC voltage at various frequencies. The frequencies for the operation are in the range of a few kHz. The system is capable of generating electric field between the two metal electrodes discharge system. The characteristics of plasma produced were measured by optical emission spectroscopy (OES) technique where electron temperature (T{sub e}) and electron number density (n{sub e}) canmore » be determined by line intensity ratio method. The value of electron number density was then determined from the Saha-Eggert equation. Our results show that the electron number density of the discharge obtained is of the order of 10{sup −17} − 10{sup −18} m{sup −3} where the electron temperature is between 1.00−2.00 eV for various operating frequencies used which are in good agreement with similar results published earlier.« less

Ozone and dinitrogen monoxide production in atmospheric pressure air dielectric barrier discharge plasma effluent generated by nanosecond pulse superimposed alternating current voltage

NASA Astrophysics Data System (ADS)

Takashima, Keisuke; Kaneko, Toshiro

2017-06-01

The effects of nanosecond pulse superposition to alternating current voltage (NS + AC) on the generation of an air dielectric barrier discharge (DBD) plasma and reactive species are experimentally studied, along with measurements of ozone (O3) and dinitrogen monoxide (N2O) in the exhausted gas through the air DBD plasma (air plasma effluent). The charge-voltage cycle measurement indicates that the role of nanosecond pulse superposition is to induce electrical charge transport and excess charge accumulation on the dielectric surface following the nanosecond pulses. The densities of O3 and N2O in NS + AC DBD are found to be significantly increased in the plasma effluent, compared to the sum of those densities generated in NS DBD and AC DBD operated individually. The production of O3 and N2O is modulated significantly by the phase in which the nanosecond pulse is superimposed. The density increase and modulation effects by the nanosecond pulse are found to correspond with the electrical charge transport and the excess electrical charge accumulation induced by the nanosecond pulse. It is suggested that the electrical charge transport by the nanosecond pulse might result in the enhancement of the nanosecond pulse current, which may lead to more efficient molecular dissociation, and the excess electrical charge accumulation induced by the nanosecond pulse increases the discharge coupling power which would enhance molecular dissociation.

Langmuir Probe Analysis of Maser-Driven Alfven Waves Using New LaB6 Cathode in LaPD

NASA Astrophysics Data System (ADS)

Clark, Mary; Dorfman, Seth; Zhu, Ziyan; Rossi, Giovanni; Carter, Troy

2015-11-01

Previous research in the Large Plasma Device shows that specific conditions on the magnetic field and cathode discharge voltage allow an Alfven wave to develop in the cathode-anode region. When the speed of bulk electrons (dependent on discharge voltage) entering the region exceeds the Alfven speed, the electrons can excite a wave. This phenomenon mimics one proposed to exist in the Earth's ionosphere. Previous experiments used a cathode coated with Barium Oxide, and this project uses a new cathode coated with Lanthanum Hexaboride (LaB6). The experiment seeks to characterize the behavior of plasmas generated with the LaB6 source, as well as understand properties of the driven wave when using the new cathode. Langmuir probes are used to find electron temperature, ion saturation current, and plasma density. These parameters determine characteristics of the wave. Preliminary analysis implies that density increases with LaB6 discharge voltage until 170 V, where it levels off. A linear increase in density is expected; the plateau implies cathode power does not ionize the plasma after 170 V. It is possible the power is carried out by the generated Alfven wave, or heats the plasma or cathode. This ``missing'' power is currently under investigation. Work funded by DOE and NSF.

Nonthermal Biological Treatments Using Discharge Plasma Produced by Pulsed Power 4. Cleaning of Lakes and Marshes by Pulsed Power Produced Streamer Discharges in Water

NASA Astrophysics Data System (ADS)

Akiyama, Hidenori; Katsuki, Sunao; Namihira, Takao; Ishibashi, Kazuo; Kiyosaki, Noriaki

Pulsed power has been used to produce non-thermal plasmas in atmospheric pressure gases that generate a high electric field at the tips of streamer discharges, where high energy electrons, free radicals, ultraviolet rays, and ozone are produced. These manifestations of streamer discharges have been used in the treatment of exhaust gases, removal of volatile and toxic compounds such as dioxin, and the sterilization of microorganisms. Here, large volume streamer discharges in water are described. These streamer discharges in liquids are able to produce a high electric field, high energy electrons, ozone, chemically active species, ultraviolet rays, and shock waves, which readily sterilize microorganisms and decompose molecules and materials. An application of this phenomenon to the cleaning of lakes and marshes is also described.

Electron series resonance in a magnetized 13.56 MHz symmetric capacitive coupled discharge

NASA Astrophysics Data System (ADS)

Joshi, J. K.; Binwal, S.; Karkari, S. K.; Kumar, Sunil

2018-03-01

A 13.56 MHz capacitive coupled radio-frequency (RF) argon discharge under transverse magnetic field has been investigated. The discharge is operated in a push-pull mode using a 1:1 isolation transformer with its centre tap grounded to a RF generator. The power delivered to the plasma has been calculated from phase-calibrated RF current/voltage waveforms measured on the secondary side of the isolation transformer. An equivalent electrical circuit of the discharge has been described to determine the net plasma impedance. It is found that in the presence of magnetic field, the discharge impedance exhibits a series resonance as the RF power level is increased gradually. However, in the un-magnetized case, the discharge remains entirely capacitive. A qualitative discussion has been given to explain the role of external magnetic field in achieving the series resonance.

Effect of Coulomb Collisions on Low Gas Pressure Plasmas

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nanbu, K.; Furubayashi, T.

2006-05-05

A recent trend in material processing plasmas is the use of a low gas pressure and high plasma density. In such plasmas, Coulomb collisions among charged particles has been considered to have a significant effect on plasma structure. By use of Bobylev and Nanbu's theory [Phy. Rev. E, 61(2000), 4576], this effect on argon plasmas and oxygen plasmas generated by a capacitive discharge is examined. It is found that the effect is appreciable only for oxygen plasmas.

Overview of recent experimental results from the Aditya tokamak

NASA Astrophysics Data System (ADS)

Tanna, R. L.; Ghosh, J.; Chattopadhyay, P. K.; Raj, Harshita; Patel, Sharvil; Dhyani, P.; Gupta, C. N.; Jadeja, K. A.; Patel, K. M.; Bhatt, S. B.; Panchal, V. K.; Patel, N. C.; Chavda, Chhaya; Praveenlal, E. V.; Shah, K. S.; Makawana, M. N.; Jha, S. K.; Gopalkrishana, M. V.; Tahiliani, K.; Sangwan, Deepak; Raju, D.; Nagora, Umesh; Pathak, S. K.; Atrey, P. K.; Purohit, S.; Raval, J.; Joisa, Y. S.; Rao, C. V. S.; Chowdhuri, M. B.; Banerjee, S.; Ramaiya, N.; Manchanda, R.; Thomas, J.; Kumar, Ajai; Ajay, Kumar; Sharma, P. K.; Kulkarni, S. V.; Sathyanarayana, K.; Shukla, B. K.; Das, Amita; Jha, R.; Saxena, Y. C.; Sen, A.; Kaw, P. K.; Bora, D.; the ADITYA Team

2017-10-01

Several experiments, related to controlled thermonuclear fusion research and highly relevant for large size tokamaks, including ITER, have been carried out in ADITYA, an ohmically heated circular limiter tokamak. Repeatable plasma discharges of a maximum plasma current of ~160 kA and discharge duration beyond ~250 ms with a plasma current flattop duration of ~140 ms have been obtained for the first time in ADITYA. The reproducibility of the discharge reproducibility has been improved considerably with lithium wall conditioning, and improved plasma discharges are obtained by precisely controlling the position of the plasma. In these discharges, chord-averaged electron density ~3.0-4.0  ×  1019 m-3 using multiple hydrogen gas puffs, with a temperature of the order of ~500-700 eV, have been achieved. Novel experiments related to disruption control are carried out and disruptions, induced by hydrogen gas puffing, are successfully mitigated using the biased electrode and ion cyclotron resonance pulse techniques. Runaway electrons are successfully mitigated by applying a short local vertical field (LVF) pulse. A thorough disruption database has been generated by identifying the different categories of disruption. Detailed analysis of several hundred disrupted discharges showed that the current quench time is inversely proportional to the q edge. Apart from this, for volt-sec recovery during the plasma formation phase, low loop voltage start-up and current ramp-up experiments have been carried out using electron cyclotron resonance heating (ECRH). Successful recovery of volt-sec leads to the achievement of longer plasma discharge durations. In addition, the neon gas puff assisted radiative improved confinement mode has also been achieved in ADITYA. All of the above mentioned experiments will be discussed in this paper.

Impact of electrode geometry on an atmospheric pressure surface barrier discharge

NASA Astrophysics Data System (ADS)

Hasan, M. I.; Morabit, Y.; Dickenson, A.; Walsh, J. L.

2017-06-01

Several of the key characteristics of an atmospheric pressure surface barrier discharge (SBD) are heavily dependent on the geometrical configuration of the plasma generating electrodes. This paper reveals that increasing the surface area of an SBD device by reducing the gaps within the electrodes can have major and unforeseen consequence on the discharge properties. It is experimentally demonstrated that a critical limit exists when reducing the diameter of a circular electrode gap below 5 mm, beyond which the required breakdown voltage increases exponentially and the power deposited in the discharge is impeded. Using a numerical model, it is shown that a reduced electrode gap diameter yields a decrease in the voltage difference between the electrode and dielectric surface, thus lowering the maximum electric field. This study indicates a link between the electrode geometry and the nature of the reactive chemistry produced in the plasma, findings which have wide-reaching implications for many applications where multiple closely packed surface barrier discharges are employed to achieve uniform and large area plasma processing.

Optical and application study of gas-liquid discharge excited by bipolar nanosecond pulse in atmospheric air.

PubMed

Wang, Sen; Wang, Wen-chun; Yang, De-zheng; Liu, Zhi-jie; Zhang, Shuai

2014-10-15

In this study, a bipolar nanosecond pulse with 20ns rising time is employed to generate air gas-liquid diffuse discharge plasma with room gas temperature in quartz tube at atmospheric pressure. The image of the discharge and optical emission spectra of active species in the plasma are recorded. The plasma gas temperature is determined to be approximately 390K by compared the experimental spectra with the simulated spectra, which is slightly higher than the room temperature. The result indicated that the gas temperature rises gradually with pulse peak voltage increasing, while decreases slightly with the electrode gap distance increasing. As an important application, bipolar nanosecond pulse discharge is used to sterilize the common microorganisms (Actinomycetes, Candida albicans and Escherichia coli) existing in drinking water, which performs high sterilization efficiency. Copyright © 2014 Elsevier B.V. All rights reserved.

Diagnosis of a short-pulse dielectric barrier discharge at atmospheric pressure in helium with hydrogen-methane admixtures

NASA Astrophysics Data System (ADS)

Nastuta, A. V.; Pohoata, V.; Mihaila, I.; Topala, I.

2018-04-01

In this study, we present results from electrical, optical, and spectroscopic diagnosis of a short-pulse (250 ns) high-power impulse (up to 11 kW) dielectric barrier discharge at atmospheric pressure running in a helium/helium-hydrogen/helium-hydrogen-methane gas mixture. This plasma source is able to generate up to 20 cm3 of plasma volume, pulsed in kilohertz range. The plasma spatio-temporal dynamics are found to be developed in three distinct phases. All the experimental observations reveal a similar dynamic to medium power microsecond barrier discharges, although the power per pulse and current density are up to two orders of magnitude higher than the case of microsecond barrier discharges. This might open the possibility for new applications in the field of gas or surface processing, and even life science. These devices can be used in laboratory experiments relevant for molecular astrophysics.

Characteristics of chiral plasma plumes generated in the absence of external magnetic field

NASA Astrophysics Data System (ADS)

Nie, LanLan; Liu, FengWu; Zhou, XinCai; Lu, XinPei; Xian, YuBin

2018-05-01

A chiral plasma plume has recently been generated inside a dielectric tube without the use of an external magnetic field. In this paper, we seek to further study the key properties of such a chiral plume to improve our understanding of how this interesting structure is generated and controlled. The chiral plume is generated by externally mounting a stainless steel helical coil or a ring onto the dielectric tube. By changing the pitch of the helical coil, the pitch of the plasma plume can be controlled, with the shape of the plume following the shape of the helical coil. The addition of the helical coil significantly expands the range of parameters under which the chiral plasma plume appears. When the frequency of the applied voltage increases, additional stable discharge channels appear between the adjacent helices. The addition of two helical coils results in the formation of two chiral plasma plumes, which follow the shape of the helical coils. When a metal ring is placed on the outside of the tube, there is no chiral plasma plume between the high voltage electrode and the ring; however, a chiral plasma plume appears on the right side of the ring if the distance between the ring and the high voltage electrode is small. These findings suggest that the chiral plasma can be effectively modulated and guided using an externally mounted helical coil, which acts as the floating/actual ground to reduce the impedance of the discharge and as such contributes to the emergence of the chiral plasma plume behavior.

Aerospace Applications of Non-Equilibrium Plasma

NASA Technical Reports Server (NTRS)

Blankson, Isaiah M.

2016-01-01

Nonequilibrium plasma/non-thermal plasma/cold plasmas are being used in a wide range of new applications in aeronautics, active flow control, heat transfer reduction, plasma-assisted ignition and combustion, noise suppression, and power generation. Industrial applications may be found in pollution control, materials surface treatment, and water purification. In order for these plasma processes to become practical, efficient means of ionization are necessary. A primary challenge for these applications is to create a desired non-equilibrium plasma in air by preventing the discharge from transitioning into an arc. Of particular interest is the impact on simulations and experimental data with and without detailed consideration of non-equilibrium effects, and the consequences of neglecting non-equilibrium. This presentation will provide an assessment of the presence and influence of non-equilibrium phenomena for various aerospace needs and applications. Specific examples to be considered will include the forward energy deposition of laser-induced non-equilibrium plasmoids for sonic boom mitigation, weakly ionized flows obtained from pulsed nanosecond discharges for an annular Hall type MHD generator duct for turbojet energy bypass, and fundamental mechanisms affecting the design and operation of novel plasma-assisted reactive systems in dielectric liquids (water purification, in-pipe modification of fuels, etc.).

On the boundary flow using pulsed nanosecond DBD plasma actuators

NASA Astrophysics Data System (ADS)

Zhao, Zi-Jie; Cui, Y. D.; Li, Jiun-Ming; Zheng, Jian-Guo; Khoo, B. C.

2018-05-01

Our previous studies in quiescent air environment [Z. J. Zhao et al., AIAA J. 53(5) (2015) 1336; J. G. Zheng et al., Phys. Fluids 26(3) (2014) 036102] reveal experimentally and numerically that the shock wave generated by the nanosecond pulsed plasma is fundamentally a microblast wave. The shock-induced burst perturbations (overpressure and induced velocity) are found to be restricted to a very narrow region (about 1 mm) behind the shock front and last only for a few microseconds. These results indicate that the pulsed nanosecond dielectric barrier discharge (DBD) plasma actuator has stronger local effects in time and spatial domain. In this paper, we further investigate the effects of pulsed plasma on the boundary layer flow over a flat plate. The present investigation reveals that the nanosecond pulsed plasma actuator generates intense perturbations and tends to promote the laminar boundary over a flat plate to turbulent flow. The heat effect after the pulsed plasma discharge was observed in the external flow, lasting a few milliseconds for a single pulse and reaching a quasi-stable state for multi-pulses.

Study of magnetic field expansion using a plasma generator for space radiation active protection

NASA Astrophysics Data System (ADS)

Jia, Xiang-Hong; Jia, Shao-Xia; Xu, Feng; Bai, Yan-Qiang; Wan, Jun; Liu, Hong-Tao; Jiang, Rui; Ma, Hong-Bo; Wang, Shou-Guo

2013-09-01

There are many active protecting methods including Electrostatic Fields, Confined Magnetic Field, Unconfined Magnetic Field and Plasma Shielding etc. for defending the high-energy solar particle events (SPE) and Galactic Cosmic Rays (GCR) in deep space exploration. The concept of using cold plasma to expand a magnetic field is the best one of all possible methods so far. The magnetic field expansion caused by plasma can improve its protective efficiency of space particles. One kind of plasma generator has been developed and installed into the cylindrical permanent magnet in the eccentric. A plasma stream is produced using a helical-shaped antenna driven by a radio-frequency (RF) power supply of 13.56 MHz, which exits from both sides of the magnet and makes the magnetic field expand on one side. The discharging belts phenomenon is similar to the Earth's radiation belt, but the mechanism has yet to be understood. A magnetic probe is used to measure the magnetic field expansion distributions, and the results indicate that the magnetic field intensity increases under higher increments of the discharge power.

Numerical study of the flow structures in flat plate and the wall-mounted hump induced by the unsteady DBD plasma

NASA Astrophysics Data System (ADS)

Yu, Jianyang; Liu, Huaping; Wang, Ruoyu; Chen, Fu

2017-01-01

In this work, the dielectric-barrier-discharge plasma actuator was employed to study the flow structures induced by the plasma actuator over a flat plate and a wall-mounted hump. A phenomenological dielectric-barrier-discharge plasma model which regarded the plasma effect as the body force was implemented into the Navier-Stokes equations solved by the method of large eddy simulations. The results show that a series of vortex pairs, which indicated dipole formation and periodicity distribution were generated in the boundary layer when the plasma was applied to the flow over a flat plane. They would enhance the energy exchanged between the near wall region and the free stream. Besides, their spatial trajectories are deeply affected by the actuation strength. When the actuator was engaged in the flow over a wall-mounted hump, the vortex pairs were also produced, which was able to delay flow separation as well as to promote flow reattachment and reduce the generation of a vortex, achieving the goal of reducing dissipation and decreasing flow resistance.

Characteristics of plasma in culture medium generated by positive pulse voltage and effects of organic compounds on its characteristics

NASA Astrophysics Data System (ADS)

Sato, Y.; Sato, T.; Yoshino, D.

2016-12-01

We describe a positive pulse voltage method for generating plasma in culture medium with a composition similar to biological fluids. We also describe the plasma’s characteristics, liquid quality, and the effect of organic compounds in the culture medium on the plasma characteristics through comparisons to a solution containing inorganic salts at the same concentrations as in the culture medium. Light emission with Na and OH spectra was observed within a vapor bubble produced by Joule heating at the tip of the electrode. A downward thermal flow and shock wave were caused by the behavior of the vapor bubble. The culture medium pH gradually increased from 7.9 to 8.3 over the discharge time of 300 s. H2O2 was generated 1.1 mg l-1 in the culture medium after discharge for 300 s, and this value was 0.5 mg l-1 lower than the inorganic salts solution which does not contain organic compounds. This study provides important data that will help facilitate more widespread application of plasma medicine.

Boron ion beam generation utilizing lanthanum hexaboride cathodes: Comparison of vacuum arc and planar magnetron glow

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nikolaev, A. G.; Vizir, A. V.; Yushkov, G. Yu., E-mail: gyushkov@mail.ru

Boron ion beams are widely used for semiconductor ion implantation and for surface modification for improving the operating parameters and increasing the lifetime of machine parts and tools. For the latter application, the purity requirements of boron ion beams are not as stringent as for semiconductor technology, and a composite cathode of lanthanum hexaboride may be suitable for the production of boron ions. We have explored the use of two different approaches to boron plasma production: vacuum arc and planar high power impulse magnetron in self-sputtering mode. For the arc discharge, the boron plasma is generated at cathode spots, whereasmore » for the magnetron discharge, the main process is sputtering of cathode material. We present here the results of comparative test experiments for both kinds of discharge, aimed at determining the optimal discharge parameters for maximum yield of boron ions. For both discharges, the extracted ion beam current reaches hundreds of milliamps and the fraction of boron ions in the total extracted ion beam is as high as 80%.« less

Low-Temperature Sterilization with Surface-Wave-Excited Oxygen Plasma

NASA Astrophysics Data System (ADS)

Nagatsu, Masaaki; Terashita, Fumie; Koide, Yukio

2003-07-01

Low-temperature plasma sterilization has been experimentally demonstrated using surface-wave plasma excited by a 2.45 GHz microwave. With the spores of Bacillus stearothermophilus and Bacillus subtilis as biological indicators, we have carried out the plasma sterilization experiments by varying the irradiation period of oxygen plasma discharges. It was experimentally confirmed that the spores with a population of 1.5 × 106 were sterilized by irradiating them with oxygen plasma discharges generated with a microwave power of 700 W at a pressure of 60-80 mTorr for 3 min or longer. From the scanning electron microscopy (SEM) analysis of the spores, we found that the sterilized spores clearly had different sizes and shapes compared with those before the plasma irradiation. Furthermore, present experiments suggested that the changes of spore shapes were mainly attributed to the reactive interactions with oxygen radicals.

Collisional and radiative processes in high-pressure discharge plasmas

NASA Astrophysics Data System (ADS)

Becker, Kurt H.; Kurunczi, Peter F.; Schoenbach, Karl H.

2002-05-01

Discharge plasmas at high pressures (up to and exceeding atmospheric pressure), where single collision conditions no longer prevail, provide a fertile environment for the experimental study of collisions and radiative processes dominated by (i) step-wise processes, i.e., the excitation of an already excited atomic/molecular state and by (ii) three-body collisions leading, for instance, to the formation of excimers. The dominance of collisional and radiative processes beyond binary collisions involving ground-state atoms and molecules in such environments allows for many interesting applications of high-pressure plasmas such as high power lasers, opening switches, novel plasma processing applications and sputtering, absorbers and reflectors for electromagnetic waves, remediation of pollutants and waste streams, and excimer lamps and other noncoherent vacuum-ultraviolet light sources. Here recent progress is summarized in the use of hollow cathode discharge devices with hole dimensions in the range 0.1-0.5 mm for the generation of vacuum-ultraviolet light.

Comparison between off-resonance and electron Bernstein waves heating regime in a microwave discharge ion source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Castro, G.; Di Giugno, R.; Miracoli, R.

2012-02-15

A microwave discharge ion source (MDIS) operating at the Laboratori Nazionali del Sud of INFN, Catania has been used to compare the traditional electron cyclotron resonance (ECR) heating with an innovative mechanisms of plasma ignition based on the electrostatic Bernstein waves (EBW). EBW are obtained via the inner plasma electromagnetic-to-electrostatic wave conversion and they are absorbed by the plasma at cyclotron resonance harmonics. The heating of plasma by means of EBW at particular frequencies enabled us to reach densities much larger than the cutoff ones. Evidences of EBW generation and absorption together with X-ray emissions due to high energy electronsmore » will be shown. A characterization of the discharge heating process in MDISs as a generalization of the ECR heating mechanism by means of ray tracing will be shown in order to highlight the fundamental physical differences between ECR and EBW heating.« less

Plasma-enhanced mixing and flameholding in supersonic flow.

PubMed

Firsov, Alexander; Savelkin, Konstantin V; Yarantsev, Dmitry A; Leonov, Sergey B

2015-08-13

The results of experimental study of plasma-based mixing, ignition and flameholding in a supersonic model combustor are presented in the paper. The model combustor has a length of 600 mm and cross section of 72 mm width and 60 mm height. The fuel is directly injected into supersonic airflow (Mach number M=2, static pressure P(st)=160-250 Torr) through wall orifices. Two series of tests are focused on flameholding and mixing correspondingly. In the first series, the near-surface quasi-DC electrical discharge is generated by flush-mounted electrodes at electrical power deposition of W(pl)=3-24 kW. The scope includes parametric study of ignition and flame front dynamics, and comparison of three schemes of plasma generation: the first and the second layouts examine the location of plasma generators upstream and downstream from the fuel injectors. The third pattern follows a novel approach of combined mixing/ignition technique, where the electrical discharge distributes along the fuel jet. The last pattern demonstrates a significant advantage in terms of flameholding limit. In the second series of tests, a long discharge of submicrosecond duration is generated across the flow and along the fuel jet. A gasdynamic instability of thermal cavity developed after a deposition of high-power density in a thin plasma filament promotes the air-fuel mixing. The technique studied in this work has weighty potential for high-speed combustion applications, including cold start/restart of scramjet engines and support of transition regime in dual-mode scramjet and at off-design operation. © 2015 The Author(s) Published by the Royal Society. All rights reserved.

Discharge mode transition and temporal-spatial evolution of an air-water plasma jet generated by pulsating DC power

NASA Astrophysics Data System (ADS)

Lei, J.; Geng, Y.; Liu, K.; Zhu, W.; Zheng, Z.; Hu, H.

2017-12-01

In this paper, pulsating direct current air-water plasma jet, which can increase the production of •OH and decrease the temperature, is studied. The results show that the discharge mode changes in one cycle from corona discharge with steep Trichel current pulse to glow-like discharge. It is unknown whether the different discharge modes and water ratio have an effect on the transient process of the excited O and •OH production and the mechanism of plasma propagation. So, a series of experiments are done in this paper. The results show that the changing rules of both the excited state O and the discharge current reach their two peak values synchronously. And its maximum appears at the time of the first peak current value in corona mode. However, the change of the excited state •OH is different. It increases to its maximum at the time of the second peak current value in glow-like mode. Besides, the intensified charge coupled device photographs show that the luminous intensity of the discharge zone at the first peak current value in corona mode is stronger than the second peak current value in glow-like mode. At the same time, the discharge area of the former is larger than the latter. Nevertheless, with the increase in water ratio, the discharge area change reversed. Additionally, the air plasma plume propagation depends on the gas flow. The initial propagation velocity decreases with the increase in water ratio.

Spatially resolved high-resolution x-ray spectroscopy of high-current plasma-focus discharges.

PubMed

Zając, S; Rzadkiewicz, J; Rosmej, O; Scholz, M; Yongtao, Zhao; Gójska, A; Paduch, M; Zielińska, E

2010-10-01

Soft x-ray emission from a Mather-type plasma-focus device (PF-1000) operated at ∼400 kJ was measured. The high density and temperature plasma were generated by the discharge in the deuterium-argon gas mixture in the modified (high-current) plasma-focus configuration. A spherically bent mica crystal spectrograph viewing the axial output of the pinch region was used to measure the x-ray spectra. Spatially resolved spectra including the characteristic x-ray lines of highly ionized Ar and continua were recorded by means of an x-ray film. The x-ray emission of PF-1000 device was studied at different areas of the pinch.

Spatially resolved high-resolution x-ray spectroscopy of high-current plasma-focus discharges

DOE Office of Scientific and Technical Information (OSTI.GOV)

ZajaPc, S.; Rzadkiewicz, J.; Scholz, M.

Soft x-ray emission from a Mather-type plasma-focus device (PF-1000) operated at {approx}400 kJ was measured. The high density and temperature plasma were generated by the discharge in the deuterium-argon gas mixture in the modified (high-current) plasma-focus configuration. A spherically bent mica crystal spectrograph viewing the axial output of the pinch region was used to measure the x-ray spectra. Spatially resolved spectra including the characteristic x-ray lines of highly ionized Ar and continua were recorded by means of an x-ray film. The x-ray emission of PF-1000 device was studied at different areas of the pinch.

Inactivation of MS2 bacteriophage by streamer corona discharge in water.

PubMed

Lee, Changha; Kim, Jaeeun; Yoon, Jeyong

2011-02-01

Electrical discharge processes are emerging as water treatment technologies applicable to both the degradation of organic contaminants as well as inactivation of pathogens. Particularly as a disinfection technology, electrical discharge processes do not produce toxic byproducts, and effectively inactivate a wide spectrum of microorganisms by multiple lethal actions generated by the formation of plasma channels. This study demonstrates the inactivation of a virus using the streamer corona discharge process (SCDP) with MS2 phage as a surrogate. A rapid inactivation of MS2 phage (i.e., approximately 4 log inactivation in 5 min) was observed in all experimental runs conducted. Discharge conditions such as applied voltage and storage capacitance significantly affected the inactivation efficiency of MS2 phage, whereas the influence of water quality parameters was minor. In order to elucidate the mechanism of MS2 phage inactivation, potentially lethal factors that can be generated by the SCDP were selected, and their roles in the inactivation of MS2 phage were examined. As a result, effects of UV radiation, chemical oxidants, and pulsed electric fields were found to be insignificant. The shockwave generated upon plasma channel formation appears to be the most important factor responsible for MS2 phage inactivation. Copyright © 2010 Elsevier Ltd. All rights reserved.

Plasma Structure and Behavior of Miniature Ring-Cusp Discharges

NASA Astrophysics Data System (ADS)

Mao, Hann-Shin

Miniature ring-cusp ion thrusters provide a unique blend of high efficiencies and millinewton level thrust for future spacecraft. These thrusters are attractive as a primary propulsion for small satellites that require a high delta V, and as a secondary propulsion for larger spacecraft that require precision formation flying, disturbance rejection, or attitude control. To ensure desirable performance throughout the life of such missions, an advancement in the understanding of the plasma structure and behavior of miniature ring-cusp discharges is required. A research model was fabricated to provide a simplified experimental test bed for the analysis of the plasma discharge chamber of a miniature ion thruster. The plasma source allowed for spatially resolved measurements with a Langmuir probe along a meridian plane. Probe measurements yielded plasma density, electron temperature, and plasma potential data. The magnetic field strength was varied along with the discharge current to determine the plasma behavior under various conditions. The structure of the plasma properties were found to be independent of the discharge power under the proper scaling. It was concluded that weaker magnetic fields can improve the overall performance for ion thruster operation. To further analyze the experimental measurements, a framework was developed based on the magnetic field. A flux aligned coordinate system was developed to decouple the perpendicular and parallel plasma motion with respect to the magnetic field. This was done using the stream function and magnetic scalar potential. Magnetic formulae provided intuition on the field profiles dependence on magnet dimensions. The flux aligned coordinate system showed that the plasma was isopycnic along constant stream function values. This was used to develop an empirical relation suitable for estimating the spatial behavior and to determine the plasma volume and loss areas. The plasma geometry estimates were applied to a control volume analysis on the plasma electrons. Balancing the plasma electron generation and loss yielded nominal values used in miniature ion thrusters. This result was ultimately used to develop a design tool for miniature discharges. This tool was used to perform a parametric evaluation on the magnet field configuration of the research mode. By understanding the plasma behavior, significant improvements over the baseline configuration were obtained with relatively minor changes, thus revealing the importance of plasma structure on the performance of miniature ring-cusp discharges.

Polymerization of phenol by using discharged plasma under hydrothermal state

NASA Astrophysics Data System (ADS)

Mitsugi, M.; Yoshida, A.; Watanabe, H.; Kiyan, T.; Takade, M.; Miyaji, K.; Namihira, T.; Kuwahara, Y.; Akiyama, H.; Hara, M.; Sasaki, M.; Goto, M.

2010-03-01

Supercritical fluid with plasma is a type of green processing media because this technique does not use catalyst and toxic solvents. In this study, we carried out experiments of organic materials in the presence of discharged plasma in sub- and supercritical water to evaluate the possibility for new reactions. For this purpose, we used SUS316 reactor that generates plasma at temperature and pressure up to 573K and 30MPa, respectively. 100 mmol/L aqueous phenol solution was used as starting material. The reactions were carried out at temperature of 523K and under pressure of 25MPa. After a series of reactions, water-soluble, water-insoluble (oily products), solid residue and gaseous product were obtained. For the analysis of these products, HPLC, GC-MS, TOC, GC-TCD and TOF-MS were used. The highest phenol conversion was 16.96% obtained at 523K, 25MPa and with 4000 times discharged plasma. Polymerized phenol was obtained as a product.

Electrical model of cold atmospheric plasma gun

NASA Astrophysics Data System (ADS)

Slutsker, Ya. Z.; Semenov, V. E.; Krasik, Ya. E.; Ryzhkov, M. A.; Felsteiner, J.; Binenbaum, Y.; Gil, Z.; Shtrichman, R.; Cohen, J. T.

2017-10-01

We present an analytical model of cold atmospheric plasma formed by a dielectric barrier discharge (DBD), which is based on the lumped and distributed elements of an equivalent electric circuit of this plasma. This model is applicable for a wide range of frequencies and amplitudes of the applied voltage pulses, no matter whether or not the generated plasma plume interacts with a target. The model allows quantitative estimation of the plasma plume length and the energy delivered to the plasma. Also, the results of this model can be used for the design of DBD guns which efficiently generate cold atmospheric plasma. A comparison of the results of the model with those obtained in experiments shows a fairly good agreement.

Method and apparatus for the formation of a spheromak plasma

DOEpatents

Yamada, Masaaki; Furth, Harold P.; Stix, Thomas H.; Todd, Alan M. M.

1982-01-01

A method and apparatus for forming a detached, compact toroidally shaped spheromak plasma by an inductive mechanism. A generally spheroidal vacuum vessel (1) houses a toroidally shaped flux ring or core (2) which contains poloidal and toroidal field generating coils. A plasma discharge occurs with the pulsing of the toroidal field coil, and the plasma is caused to expand away from the core (2) and toward the center of the vacuum vessel (1). When the plasma is in an expanded state, a portion of it is pinched off in order to form a separate, detached spheromak plasma configuration. The detached plasma is supported by a magnetic field generated by externally arranged equilibrium field coils (5).

Energy efficiency in nanoscale synthesis using nanosecond plasmas

PubMed Central

Pai, David Z.; (Ken) Ostrikov, Kostya; Kumar, Shailesh; Lacoste, Deanna A.; Levchenko, Igor; Laux, Christophe O.

2013-01-01

We report a nanoscale synthesis technique using nanosecond-duration plasma discharges. Voltage pulses 12.5 kV in amplitude and 40 ns in duration were applied repetitively at 30 kHz across molybdenum electrodes in open ambient air, generating a nanosecond spark discharge that synthesized well-defined MoO3 nanoscale architectures (i.e. flakes, dots, walls, porous networks) upon polyamide and copper substrates. No nitrides were formed. The energy cost was as low as 75 eV per atom incorporated into a nanostructure, suggesting a dramatic reduction compared to other techniques using atmospheric pressure plasmas. These findings show that highly efficient synthesis at atmospheric pressure without catalysts or external substrate heating can be achieved in a simple fashion using nanosecond discharges. PMID:23386976

Historical Overview of Directed-Energy Work at Dahlgren

DTIC Science & Technology

2012-01-01

discharge of electrical energy at the gun breech to generate a plasma jet. This plasma jet heated a low- molecular-weight working fluid, such as water, to...cept augmented the electrical energy generating the plasma jet with a chemical reaction. A 127mm ETC gun was investigated, and a 60mm ETC gun was...ANSI Std Z39-18 13 Historical Overview of Directed-Energy Work at Dahlgren coaxial pipe, which was switched at one end, to create the oscillating

High-voltage electrode optimization towards uniform surface treatment by a pulsed volume discharge

NASA Astrophysics Data System (ADS)

Ponomarev, A. V.; Pedos, M. S.; Scherbinin, S. V.; Mamontov, Y. I.; Ponomarev, S. V.

2015-11-01

In this study, the shape and material of the high-voltage electrode of an atmospheric pressure plasma generation system were optimised. The research was performed with the goal of achieving maximum uniformity of plasma treatment of the surface of the low-voltage electrode with a diameter of 100 mm. In order to generate low-temperature plasma with the volume of roughly 1 cubic decimetre, a pulsed volume discharge was used initiated with a corona discharge. The uniformity of the plasma in the region of the low-voltage electrode was assessed using a system for measuring the distribution of discharge current density. The system's low-voltage electrode - collector - was a disc of 100 mm in diameter, the conducting surface of which was divided into 64 radially located segments of equal surface area. The current at each segment was registered by a high-speed measuring system controlled by an ARM™-based 32-bit microcontroller. To facilitate the interpretation of results obtained, a computer program was developed to visualise the results. The program provides a 3D image of the current density distribution on the surface of the low-voltage electrode. Based on the results obtained an optimum shape for a high-voltage electrode was determined. Uniformity of the distribution of discharge current density in relation to distance between electrodes was studied. It was proven that the level of non-uniformity of current density distribution depends on the size of the gap between electrodes. Experiments indicated that it is advantageous to use graphite felt VGN-6 (Russian abbreviation) as the material of the high-voltage electrode's emitting surface.

Effect of turbulent flow on an atmospheric-pressure AC powered gliding arc discharge

NASA Astrophysics Data System (ADS)

Kong, Chengdong; Gao, Jinlong; Zhu, Jiajian; Ehn, Andreas; Aldén, Marcus; Li, Zhongshan

2018-06-01

A high-power gliding arc (GA) discharge was generated in a turbulent air flow driven by a 35 kHz alternating current electric power supply. The effects of the flow rate on the characteristics of the GA discharge were investigated using combined optical and electrical diagnostics. Phenomenologically, the GA discharge exhibits two types of discharge, i.e., glow type and spark type, depending on the flow rates and input powers. The glow-type discharge, which has peak currents of hundreds of milliamperes, is sustained at low flow rates. The spark-type discharge, which is characterized by a sharp current spike of several amperes with duration of less than 1 μs, occurs more frequently as the flow rate increases. Higher input power can suppress spark-type discharges in moderate turbulence, but this effect becomes weak under high turbulent conditions. Physically, the transition between glow- and spark-type is initiated by the short cutting events and the local re-ignition events. Short cutting events occur owing to the twisting, wrinkling, and stretching of the plasma columns that are governed by the relatively large vortexes in the flow. Local re-ignition events, which are defined as re-ignition along plasma columns, are detected in strong turbulence due to increment of the impedance of the plasma column and consequently the internal electric field strength. It is suggested that the vortexes with length scales smaller than the size of the plasma can penetrate into the plasma column and promote mixing with surroundings to accelerate the energy dissipation. Therefore, the turbulent flow influences the GA discharges by ruling the short cutting events with relatively large vortexes and the local re-ignition events with small vortexes.

Activation of peroxydisulfate by gas-liquid pulsed discharge plasma to enhance the degradation of p-nitrophenol

NASA Astrophysics Data System (ADS)

Shang, Kefeng; Wang, Hao; Li, Jie; Lu, Na; Jiang, Nan; Wu, Yan

2017-06-01

Pulsed discharge in water and over water surfaces generates ultraviolet radiation, local high temperature, shock waves, and chemical reactive species, including hydroxyl radicals, hydrogen peroxide, and ozone. Pulsed discharge plasma (PDP) can oxidize and mineralize pollutants very efficiently, but high energy consumption restricts its application for industrial wastewater treatment. A novel method for improving the energy efficiency of wastewater treatment by PDP was proposed, in which peroxydisulfate (PDS) was added to wastewater and PDS was activated by PDP to produce more strong oxidizing radicals, including sulfate radicals and hydroxyl radicals, leading to a higher oxidation capacity for the PDP system. The experimental results show that the increase in solution conductivity slightly decreased the discharge power of the pulse discharge over the water surface. An increase in the discharge intensity improved the activation of PDS and therefore the degradation efficiency and energy efficiency of p-nitrophenol (PNP). An increase in the addition dosage of PDS greatly facilitated the degradation of PNP at a molar ratio of PDS to PNP of lower than 80:1, but the performance enhancement was no longer obvious at a dosage of more than 80:1. Under an applied voltage of 20 kV and a gas discharge gap of 2 mm, the degradation efficiency and energy efficiency of the PNP reached 90.7% and 45.0 mg kWh-1 for the plasma/PDS system, respectively, which was 34% and 18.0 mg kWh-1 higher than for the discharge plasma treatment alone. Analysis of the physical and chemical effects indicated that ozone and hydrogen peroxide were important for PNP degradation and UV irradiation and heat from the discharge plasma might be the main physical effects for the activation of PDS.

Influence of finite geometrical asymmetry of the electrodes in capacitively coupled radio frequency plasma

NASA Astrophysics Data System (ADS)

Bora, B.; Soto, L.

2014-08-01

Capacitively coupled radio frequency (CCRF) plasmas are widely studied in last decades due to the versatile applicability of energetic ions, chemically active species, radicals, and also energetic neutral species in many material processing fields including microelectronics, aerospace, and biology. A dc self-bias is known to generate naturally in geometrically asymmetric CCRF plasma because of the difference in electrode sizes known as geometrical asymmetry of the electrodes in order to compensate electron and ion flux to each electrode within one rf period. The plasma series resonance effect is also come into play due to the geometrical asymmetry and excited several harmonics of the fundamental in low pressure CCRF plasma. In this work, a 13.56 MHz CCRF plasma is studied on the based on the nonlinear global model of asymmetric CCRF discharge to understand the influences of finite geometrical asymmetry of the electrodes in terms of generation of dc self-bias and plasma heating. The nonlinear global model on asymmetric discharge has been modified by considering the sheath at the grounded electrode to taking account the finite geometrical asymmetry of the electrodes. The ion density inside both the sheaths has been taken into account by incorporating the steady-state fluid equations for ions considering that the applied rf frequency is higher than the typical ion plasma frequency. Details results on the influences of geometrical asymmetry on the generation of dc self-bias and plasma heating are discussed.

Piezoelectric transformers for low-voltage generation of gas discharges and ionic winds in atmospheric air

DOE Office of Scientific and Technical Information (OSTI.GOV)

Johnson, Michael J.; Go, David B., E-mail: dgo@nd.edu; Department of Chemical and Biomolecular Engineering, University of Notre Dame, Notre Dame, Indianapolis 46556

To generate a gas discharge (plasma) in atmospheric air requires an electric field that exceeds the breakdown threshold of ∼30 kV/cm. Because of safety, size, or cost constraints, the large applied voltages required to generate such fields are often prohibitive for portable applications. In this work, piezoelectric transformers are used to amplify a low input applied voltage (<30 V) to generate breakdown in air without the need for conventional high-voltage electrical equipment. Piezoelectric transformers (PTs) use their inherent electromechanical resonance to produce a voltage amplification, such that the surface of the piezoelectric exhibits a large surface voltage that can generate corona-like dischargesmore » on its corners or on adjacent electrodes. In the proper configuration, these discharges can be used to generate a bulk air flow called an ionic wind. In this work, PT-driven discharges are characterized by measuring the discharge current and the velocity of the induced ionic wind with ionic winds generated using input voltages as low as 7 V. The characteristics of the discharge change as the input voltage increases; this modifies the resonance of the system and subsequent required operating parameters.« less

Study on the characteristics of a two gap capillary discharge

DOE Office of Scientific and Technical Information (OSTI.GOV)

Huang, D.; Yang, L. J., E-mail: yanglj@mail.xjtu.edu.cn; Huo, P.

2015-02-15

The paper presents a new two-gap capillary (TGC) discharge structure. The prominent innovation is the introduction of the middle electrode, which divides the capillary into the trigger gap and the main gap. The discharge circuit of the TGC comprises the trigger circuit and the main circuit. The two circuits are used for the pre-ionization of the trigger gap and providing energy of 450 J for the main gap arc discharging, respectively. When the discharge initiates, the trigger gap is pre-ionized under high voltage pulse produced by trigger circuit, and meanwhile, the weakly ionized plasma is generated. The main circuit then maintainsmore » the expansion of the plasma, which is called soft capillary discharge. Afterwards, the main gap is shorted and discharges under a relatively low voltage. With the optimization of the circuit parameter, both the energy deposition ratio in main gap and the degree of plasma ionization are enhanced. The efficiency of the energy deposition is almost twice higher compared with that of the conventional capillary structure. The life performance test indicates that the erosion of the middle electrode and the trigger gap carbonization are the key factors that limit the life performance of the TGC.« less

Correlation of the neutron yield from the plasma focus upon variations in the magnetic field energy of the discharge circuit

NASA Astrophysics Data System (ADS)

Ablesimov, V. E.; Dolin, Yu. N.; Kalinychev, A. E.; Tsibikov, Z. S.

2017-10-01

The relation between neutron yield Y and magnetic field energy variations Δ W in the discharge circuit has been studied for a Mather-type plasma-focus camera. The activation technique (activation of silver isotopes) has been used to measure the integral yield of DD neutrons from the source. The time dependence of the neutron yield has been recorded by scintillation detectors. For the device used in the investigations, the neutron yield exhibits a linear dependence on variations in the magnetic field energy Δ W in the discharge circuit at the instant of neutron generation. It is also found that this dependence is related to the initial deuteron pressure in the discharge chamber.

Laser-driven acceleration of electrons in a partially ionized plasma channel.

PubMed

Rowlands-Rees, T P; Kamperidis, C; Kneip, S; Gonsalves, A J; Mangles, S P D; Gallacher, J G; Brunetti, E; Ibbotson, T; Murphy, C D; Foster, P S; Streeter, M J V; Budde, F; Norreys, P A; Jaroszynski, D A; Krushelnick, K; Najmudin, Z; Hooker, S M

2008-03-14

The generation of quasimonoenergetic electron beams, with energies up to 200 MeV, by a laser-plasma accelerator driven in a hydrogen-filled capillary discharge waveguide is investigated. Injection and acceleration of electrons is found to depend sensitively on the delay between the onset of the discharge current and the arrival of the laser pulse. A comparison of spectroscopic and interferometric measurements suggests that injection is assisted by laser ionization of atoms or ions within the channel.

The study of low temperature plasma of pulse discharge in relation to air cleaning units.

NASA Astrophysics Data System (ADS)

Ponizovskiy, A.; Gosteev, S.; Kuzhel, O.

2017-11-01

In paper it studied parameters of low-temperature plasma (LTP) used in systems for cleaning waste gas. LTP created by positive nanosecond corona discharges, generated by high voltage pulses with a rise time of 50 ns, duration up to 400 ns, an amplitude up to 90 kV and pulses repetition 50-1000 Hz. in coaxial electrode system with gap space 3-10 cm through which moving air with linear velocity v = 0.01 to 10 m/s.

Development of a plasma focus neutron source powered by an explosive magnetic generator

NASA Astrophysics Data System (ADS)

Ablesimov, V. E.; Andrianov, A. V.; Bazanov, A. A.; Glybin, A. M.; Dolin, Yu. N.; Drozdov, I. Yu.; Drozdov, Yu. M.; Duday, P. V.; Zimenkov, A. A.; Ivanov, V. A.; Ivanovskii, A. V.; Kalinychev, A. E.; Karpov, G. V.; Kraev, A. I.; Lomtev, S. S.; Nudikov, V. N.; Pak, S. V.; Pozdov, N. I.; Polyushko, S. M.; Rybakov, A. F.; Skobelev, A. N.; Turov, A. N.; Fevralev, A. Yu.

2015-01-01

This paper presents the results of laboratory and explosive experiments with a plasma focus discharge Mather-type chamber at a discharge current amplitude of 1.3-1.4 MA. It has been found that in laboratory experiments, the yield of a deuterium-deuterium neutrons reached 1011, and in an explosive experiment using the chamber filled with a deuterium-tritium gas mixture, the integral yield of a deuterium-tritium neutrons with an energy of 14 MeV was more than 1012 neutrons.

Application of LIF technique for the space- and time-resolved monitoring of pollutant gas decomposition in nonthermal plasma reactors

NASA Astrophysics Data System (ADS)

Mizeraczyk, Jerzy; Ohkubo, Toshikazu; Kanazawa, Seiji; Kocik, Marek

2003-10-01

Laser-induced fluorescence (LIF) technique aided by intensified CCD light signal detection and fast digital image processing is demonstrated to be a useful diagnostic method for in-situ observation of the discharge-induced plasma-chemistry processes responsible for NOx(NO + NO2) decomposition occurring in non-thermal plasma reactors. In this paper a method and results of the LIF measurement of two-dimensional distribution of the ground-state NO molecule density inside a DC positive streamer corona reactor during NO removal from a flue gas simulator [air/NO(up to 300 ppm)] are presented. Either a needle-to-plate or nozzle-to-plate electrode system, having an electrode gap of 30-50 mm was used for generating the corona discharge in the reactor. The LIF monitoring of NO molecules was carried out under the steady-state DC corona discharge condition. The laser-induced fluorescence on the transition NO X2Π(v"=0)<--A2Σ+(v'=0) at λ=226nm was chosen for monitoring ground-state NO molecules in the reactor. This transition was induced by irradiation of the NO molecules with UV laser pulses generated by a laser system consisted of a XeF excimer laser, dye laser and BBO crystal. The laser pulses from the XeF excimer laser (Lambda Physik, Complex 150, λ=351 nm) pumped the dye laser (Lambda Physik, Scanmate) with Coumarin 47 as a dye, which generated the laser beam of a wavelength turned around λ=450 nm. Then, the tuned dye laser beam pumped the BBO crystal in which the second harmonic radiation of a wavelength correspondingly tuned around λ=226 nm was generated. The 226-nm UV laser pulses of energy of 0.8-2 mJ and duration of about 20 ns were transformed into the form of the so-called laser sheet (width of 1 mm, height of 30-50 mm) which passed between the electrodes through the operating gas. The obtained results, presented in the form of images, which illustrated the two-dimensional distributions of NO molecule concentration in the non-thermal reactor, showed that the corona discharge-induced removal of NO molecules occurred not only in the vicinity of the plasma region formed by the corona discharge-induced removal of NO molecules occurred not only in the vicinity of the plasma region formed by the corona streamers and in the downstream region of the reactor but also in the upstream region of the reactor, i.e. before the flue gas simulator has entered the plasma region. This information obtained owing to the LIF technique, is important for the understanding of the plasma-chemistry processes responsible for NOx decomposition in non-thermal plasma reactors and for optimising their performance.

Multiscale modeling and general theory of non-equilibrium plasma-assisted ignition and combustion

NASA Astrophysics Data System (ADS)

Yang, Suo; Nagaraja, Sharath; Sun, Wenting; Yang, Vigor

2017-11-01

A self-consistent framework for modeling and simulations of plasma-assisted ignition and combustion is established. In this framework, a ‘frozen electric field’ modeling approach is applied to take advantage of the quasi-periodic behaviors of the electrical characteristics to avoid the re-calculation of electric field for each pulse. The correlated dynamic adaptive chemistry (CO-DAC) method is employed to accelerate the calculation of large and stiff chemical mechanisms. The time-step is dynamically updated during the simulation through a three-stage multi-time scale modeling strategy, which utilizes the large separation of time scales in nanosecond pulsed plasma discharges. A general theory of plasma-assisted ignition and combustion is then proposed. Nanosecond pulsed plasma discharges for ignition and combustion can be divided into four stages. Stage I is the discharge pulse, with time scales of O (1-10 ns). In this stage, input energy is coupled into electron impact excitation and dissociation reactions to generate charged/excited species and radicals. Stage II is the afterglow during the gap between two adjacent pulses, with time scales of O (1 0 0 ns). In this stage, quenching of excited species dissociates O2 and fuel molecules, and provides fast gas heating. Stage III is the remaining gap between pulses, with time scales of O (1-100 µs). The radicals generated during Stages I and II significantly enhance exothermic reactions in this stage. The cumulative effects of multiple pulses is seen in Stage IV, with time scales of O (1-1000 ms), which include preheated gas temperatures and a large pool of radicals and fuel fragments to trigger ignition. For flames, plasma could significantly enhance the radical generation and gas heating in the pre-heat zone, thereby enhancing the flame establishment.

Removal properties of diesel exhaust particles by a dielectric barrier discharge reactor.

PubMed

Suzuki, Ken-ichiro; Takeuchi, Naomi; Madokoro, Kazuhiko; Fushimi, Chihiro; Yao, Shuiliang; Fujioka, Yuichi; Nihei, Yoshimasa

2008-02-01

The removal properties of diesel exhaust particles (DEP) were investigated using an engine exhaust particle size spectrometer (EEPS), field emission-type scanning electron microscopy (FE-SEM) and time-of-flight secondary ion mass spectrometry (TOF-SIMS). DEP were treated using a dielectric barrier discharge (DBD) reactor installed in the tail pipe of a diesel engine, and a model DBD reactor fed with DEP in the mixture of N(2) and O(2). When changing the experimental parameters of both the plasma conditions and the engine load conditions, we obtained characteristic information of DEP treated with plasma discharges from the particle diameter and the composition. In evaluating the model DBD reactor, it became clear that there were two types of plasma processes (reactions with active oxygen species to yield CO(2) and reactions with active nitrogen species to yield nitrogen containing compounds). Moreover, from the result of a TOF-SIMS analysis, the characteristic secondary ions, such as C(2)H(6)N(+), C(4)H(12)N(+), and C(10)H(20)N(2)(+), were strongly detected from the DEP surfaces during the plasma discharges. This indicates that the nitrogen contained hydrocarbons were generated by plasma reactions.

Development of plasma sources for ICRF heating experiment in KMAX mirror device

NASA Astrophysics Data System (ADS)

Sun, Xuan; Liu, Ming; Yi, Hongshen; Lin, Munan; Shi, Peiyun

2016-10-01

KMAX, Keda Mirror with AXisymmeticity, is a tandem mirror machine with a length of 10 meters and diameters of 1.2 meters in the central cell and 0.3 meters in the mirror throat. In the past experiments, the plasma was generated by helicon wave launched from the west end. We obtained the blue core mode in argon discharge, however, it cannot provide sufficient plasma for hydrogen discharge, which is at least 1012 cm-3 required for effective ICRF heating. Several attempts have thus been tried or under design to increase the central cell's plasma density: (1) a washer gun with aperture of 1cm has been successfully tested, and a plasma density of 1013 cm-3 was achieved in the west cell near the gun, however, the plasma is only 1011 cm-3 in the central cell possible due to the mirror trapping and/or neutral quenching effect (2) a larger washer gun with aperture of 2.5 cm and a higher power capacitor bank are being assembled in order to generate more plasmas. In addition, how to mitigate the neutrals is under consideration (3) A hot cathode is been designed and will be tested in combination with plasma gun or alone. Preliminary results from those plasma sources will be presented and discussed.

Method and apparatus for charged particle propagation

DOEpatents

Hershcovitch, Ady

1996-11-26

A method and apparatus are provided for propagating charged particles from a vacuum to a higher pressure region. A generator 14,14b includes an evacuated chamber 16a,b having a gun 18,18b for discharging a beam of charged particles such as an electron beam 12 or ion beam 12b. The beam 12,12b is discharged through a beam exit 22 in the chamber 16a,b into a higher pressure region 24. A plasma interface 34 is disposed at the beam exit 22 and includes a plasma channel 38 for bounding a plasma 40 maintainable between a cathode 42 and an anode 44 disposed at opposite ends thereof. The plasma channel 38 is coaxially aligned with the beam exit 22 for propagating the beam 12,12b from the chamber 16a,b, through the plasma 40, and into the higher pressure region 24. The plasma 40 is effective for pumping down the beam exit 22 for preventing pressure increase in the chamber 16a,b, and provides magnetic focusing of the beam 12,12b discharged into the higher pressure region 24.

Formation and dynamics of plasma bullets in a non-thermal plasma jet: influence of the high-voltage parameters on the plume characteristics

NASA Astrophysics Data System (ADS)

Jarrige, Julien; Laroussi, Mounir; Karakas, Erdinc

2010-12-01

Non-thermal plasma jets in open air are composed of ionization waves commonly known as 'plasma bullets' propagating at high velocities. We present in this paper an experimental study of plasma bullets produced in a dielectric barrier discharge linear-field reactor fed with helium and driven by microsecond high-voltage pulses. Two discharges were produced between electrodes for every pulse (at the rising and falling edge), but only one bullet was generated. Fast intensified charge coupled device camera imaging showed that bullet velocity and diameter increase with applied voltage. Spatially resolved optical emission spectroscopy measurements provided evidence of the hollow structure of the jet and its contraction. It was shown that the pulse amplitude significantly enhances electron energy and production of active species. The plasma bullet appeared to behave like a surface discharge in the tube, and like a positive streamer in air. A kinetics mechanism based on electron impact, Penning effect and charge transfer reactions is proposed to explain the propagation of the ionization front and temporal behavior of the radiative species.

Roles of individual radicals generated by a submerged dielectric barrier discharge plasma reactor during Escherichia coli O157:H7 inactivation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Khan, Muhammad Saiful Islam; Lee, Eun-Jung; Kim, Yun-Ji, E-mail: yunji@kfri.re.kr

A submerged dielectric barrier discharge plasma reactor (underwater DBD) has been used on Escherichia coli O157:H7 (ATCC 35150). Plasma treatment was carried out using clean dry air gas to investigate the individual effects of the radicals produced by underwater DBD on an E. coli O157:H7 suspension (8.0 log CFU/ml). E. coli O157:H7 was reduced by 6.0 log CFU/ml for 2 min of underwater DBD plasma treatment. Optical Emission Spectra (OES) shows that OH and NO (α, β) radicals, generated by underwater DBD along with ozone gas. E. coli O157:H7 were reduced by 2.3 log CFU/ml for 10 min of underwatermore » DBD plasma treatment with the terephthalic acid (TA) OH radical scavenger solution, which is significantly lower (3.7 log CFU/ml) than the result obtained without using the OH radical scavenger. A maximum of 1.5 ppm of ozone gas was produced during the discharge of underwater DBD, and the obtained reduction difference in E.coli O157:H7 in presence and in absence of ozone gas was 1.68 log CFU/ml. The remainder of the 0.62 log CFU/ml reduction might be due to the effect of the NO (α, β) radicals or due to the combined effect of all the radicals produced by underwater DBD. A small amount of hydrogen peroxide was also generated but does not play any role in E. coli O157:H7 inactivation.« less

Roles of individual radicals generated by a submerged dielectric barrier discharge plasma reactor during Escherichia coli O157:H7 inactivation

NASA Astrophysics Data System (ADS)

Khan, Muhammad Saiful Islam; Lee, Eun-Jung; Kim, Yun-Ji

2015-10-01

A submerged dielectric barrier discharge plasma reactor (underwater DBD) has been used on Escherichia coli O157:H7 (ATCC 35150). Plasma treatment was carried out using clean dry air gas to investigate the individual effects of the radicals produced by underwater DBD on an E. coli O157:H7 suspension (8.0 log CFU/ml). E. coli O157:H7 was reduced by 6.0 log CFU/ml for 2 min of underwater DBD plasma treatment. Optical Emission Spectra (OES) shows that OH and NO (α, β) radicals, generated by underwater DBD along with ozone gas. E. coli O157:H7 were reduced by 2.3 log CFU/ml for 10 min of underwater DBD plasma treatment with the terephthalic acid (TA) OH radical scavenger solution, which is significantly lower (3.7 log CFU/ml) than the result obtained without using the OH radical scavenger. A maximum of 1.5 ppm of ozone gas was produced during the discharge of underwater DBD, and the obtained reduction difference in E.coli O157:H7 in presence and in absence of ozone gas was 1.68 log CFU/ml. The remainder of the 0.62 log CFU/ml reduction might be due to the effect of the NO (α, β) radicals or due to the combined effect of all the radicals produced by underwater DBD. A small amount of hydrogen peroxide was also generated but does not play any role in E. coli O157:H7 inactivation.

Singlet oxygen generation in gas discharge for oxygen-iodine laser pumping

NASA Astrophysics Data System (ADS)

Lopaev, D. V.; Braginsky, O. V.; Klopovsky, K. S.; Kovalev, A. S.; Mankelevich, Yu. A.; Popov, N. A.; Rakhimov, A. T.; Rakhimova, T. V.; Vasilieva, A. N.

2004-09-01

The possibility of development of effective discharged singlet oxygen (SO) generator (DSOG) for oxygen-iodine laser (OIL) is studied in detail. Researches of kinetics of oxygen atoms and oxygen molecules in the lowest metastable singlet states have been carried out in the different discharges and its afterglow (DC discharges, E-beam controlled discharge and RF discharges) in both CW and pulsed mode in a wide range of conditions (pressures, gas mixtures, energy deposits etc.). The models developed for all the discharges have allowed us to analyze SO generation and loss mechanisms and to find out the key-parameters controlling the highest SO yield. It is shown that in addition to spatial plasma uniformity at low E/N and high specific energy deposit per oxygen molecule, DSOG must be oxygen atom free to avoid fast three-body quenching of SO by atomic oxygen with increasing pressure and thereby to provide pressure scaling (in tens Torrs) for applying to real OIL systems.

Effects of discharge chamber length on the negative ion generation in volume-produced negative hydrogen ion source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Chung, Kyoung-Jae; Jung, Bong-Ki; An, YoungHwa

2014-02-15

In a volume-produced negative hydrogen ion source, control of electron temperature is essential due to its close correlation with the generation of highly vibrationally excited hydrogen molecules in the heating region as well as the generation of negative hydrogen ions by dissociative attachment in the extraction region. In this study, geometric effects of the cylindrical discharge chamber on negative ion generation via electron temperature changes are investigated in two discharge chambers with different lengths of 7.5 cm and 11 cm. Measurements with a radio-frequency-compensated Langmuir probe show that the electron temperature in the heating region is significantly increased by reducingmore » the length of the discharge chamber due to the reduced effective plasma size. A particle balance model which is modified to consider the effects of discharge chamber configuration on the plasma parameters explains the variation of the electron temperature with the chamber geometry and gas pressure quite well. Accordingly, H{sup −} ion density measurement with laser photo-detachment in the short chamber shows a few times increase compared to the longer one at the same heating power depending on gas pressure. However, the increase drops significantly as operating gas pressure decreases, indicating increased electron temperatures in the extraction region degrade dissociative attachment significantly especially in the low pressure regime. It is concluded that the increase of electron temperature by adjusting the discharge chamber geometry is efficient to increase H{sup −} ion production as long as low electron temperatures are maintained in the extraction region in volume-produced negative hydrogen ion sources.« less

Microwave processes in the SPD-ATON stationary plasma thruster

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kirdyashev, K. P., E-mail: kpk@ms.ire.rssi.ru

2016-09-15

Results of experimental studies of microwave processes accompanying plasma acceleration in the SPD-ATON stationary plasma thruster are presented. Specific features of the generation of microwave oscillations in both the acceleration channel and the plasma flow outgoing from the thruster are analyzed on the basis of local measurements of the spectra of the plasma wave fields. Mechanisms for generation of microwave oscillations are considered with allowance for the inhomogeneity of the electron density and magnetic field behind the edge of the acceleration channel. The effect of microwave oscillations on the electron transport and the formation of the discharge current in themore » acceleration channel is discussed.« less

Effect of catalysts on dc corona discharge poisoning

NASA Astrophysics Data System (ADS)

Pekárek, S.

2011-02-01

The processes of ozone generation in non-thermal plasma produced by an electrical discharge in air at atmospheric pressure are burdened by the presence of nitrogen oxides, which on the one hand contribute to ozone generation and on the other hand are responsible for unpleasant discharge poisoning. The term discharge poisoning refers to the situation when the discharge ozone formation completely breaks down. Discharge poisoning can be affected by placing a catalyst in the discharge chamber. For the dc hollow needle to mesh corona discharge enhanced by the flow of air through the needle electrode we studied the effect of titanium dioxide TiO2, ZSM-5 zeolite or Cu++ZSM-5 zeolite on discharge poisoning by monitoring the ozone, nitrogen monoxide and nitrogen dioxide discharge production. We found that placing globules of any of these catalysts on the mesh decreases the energy density of the onset of discharge poisoning, and this energy density is smallest for a discharge with globules of a TiO2 on the mesh.

Application of ICP-OES for Evaluating Energy Extraction and Production Wastewater Discharge Impacts on Surface Waters in Western Pennsylvania

EPA Science Inventory

Oil and gas extraction and coal-fired electrical power generating stations produce wastewaters that are treated and discharged to rivers in Western Pennsylvania with public drinking water system (PDWS) intakes. Inductively coupled plasma optical emission spectroscopy (ICP-OES) w...

Microsecond-pulsed dielectric barrier discharge plasma stimulation of tissue macrophages for treatment of peripheral vascular disease

PubMed Central

Miller, V.; Lin, A.; Kako, F.; Gabunia, K.; Kelemen, S.; Brettschneider, J.; Fridman, G.; Fridman, A.; Autieri, M.

2015-01-01

Angiogenesis is the formation of new blood vessels from pre-existing vessels and normally occurs during the process of inflammatory reactions, wound healing, tissue repair, and restoration of blood flow after injury or insult. Stimulation of angiogenesis is a promising and an important step in the treatment of peripheral artery disease. Reactive oxygen species have been shown to be involved in stimulation of this process. For this reason, we have developed and validated a non-equilibrium atmospheric temperature and pressure short-pulsed dielectric barrier discharge plasma system, which can non-destructively generate reactive oxygen species and other active species at the surface of the tissue being treated. We show that this plasma treatment stimulates the production of vascular endothelial growth factor, matrix metalloproteinase-9, and CXCL 1 that in turn induces angiogenesis in mouse aortic rings in vitro. This effect may be mediated by the direct effect of plasma generated reactive oxygen species on tissue. PMID:26543345

Microsecond-pulsed dielectric barrier discharge plasma stimulation of tissue macrophages for treatment of peripheral vascular disease

DOE Office of Scientific and Technical Information (OSTI.GOV)

Miller, V., E-mail: vmiller@coe.drexel.edu; Lin, A.; Brettschneider, J.

Angiogenesis is the formation of new blood vessels from pre-existing vessels and normally occurs during the process of inflammatory reactions, wound healing, tissue repair, and restoration of blood flow after injury or insult. Stimulation of angiogenesis is a promising and an important step in the treatment of peripheral artery disease. Reactive oxygen species have been shown to be involved in stimulation of this process. For this reason, we have developed and validated a non-equilibrium atmospheric temperature and pressure short-pulsed dielectric barrier discharge plasma system, which can non-destructively generate reactive oxygen species and other active species at the surface of themore » tissue being treated. We show that this plasma treatment stimulates the production of vascular endothelial growth factor, matrix metalloproteinase-9, and CXCL 1 that in turn induces angiogenesis in mouse aortic rings in vitro. This effect may be mediated by the direct effect of plasma generated reactive oxygen species on tissue.« less

Coplanar surface barrier discharge ignited in water vapor—a selective source of OH radicals proved by (TA)LIF measurement

NASA Astrophysics Data System (ADS)

Procházka, V.; Tučeková, Z.; Dvořák, P.; Kováčik, D.; Slavíček, P.; Zahoranová, A.; Voráč, J.

2018-01-01

Coplanar dielectric barrier discharge (DBD) was ignited in pure water vapor at atmospheric pressure in order to generate highly oxidizing plasma with one specific type of reactive radicals. In order to prevent water condensation the used plasma reactor was heated to 120 {}\\circ C. The composition of the radical species in the discharge was studied by methods based on laser-induced fluorescence (LIF) and compared with analogous measurements realized in the same coplanar DBD ignited in air. Fast collisional processes and laser-surface interaction were taken into account during LIF data processing. It was found that coplanar DBD ignited in water vapor produces hydroxyl (OH) radicals with concentration in the order of 1020 m-3, which is 10× higher than the value measured in discharge in humid air (40% relative humidity at 21 {}\\circ C). The concentration of atomic hydrogen radicals in the DBD ignited in water vapor was below the detection limit, which proves that the generation of oxidizing plasma with dominance of one specific type of reactive radicals was achieved. The temporal evolution, spatial distribution, power dependence and rotational temperature of the OH radicals was determined in the DBD ignited in both water vapor and air.

Intense steady state electron beam generator

DOEpatents

Hershcovitch, A.; Kovarik, V.J.; Prelec, K.

1990-07-17

An intense, steady state, low emittance electron beam generator is formed by operating a hollow cathode discharge plasma source at critical levels in combination with an extraction electrode and a target electrode that are operable to extract a beam of fast primary electrons from the plasma source through a negatively biased grid that is critically operated to repel bulk electrons toward the plasma source while allowing the fast primary electrons to move toward the target in the desired beam that can be successfully transported for relatively large distances, such as one or more meters away from the plasma source. 2 figs.

Intense steady state electron beam generator

DOEpatents

Hershcovitch, Ady; Kovarik, Vincent J.; Prelec, Krsto

1990-01-01

An intense, steady state, low emittance electron beam generator is formed by operating a hollow cathode discharge plasma source at critical levels in combination with an extraction electrode and a target electrode that are operable to extract a beam of fast primary electrons from the plasma source through a negatively biased grid that is critically operated to repel bulk electrons toward the plasma source while allowing the fast primary electrons to move toward the target in the desired beam that can be successfully transported for relatively large distances, such as one or more meters away from the plasma source.

Development of double-pulse lasers ablation system for generating gold ion source under applying an electric field

NASA Astrophysics Data System (ADS)

Khalil, A. A. I.

2015-12-01

Double-pulse lasers ablation (DPLA) technique was developed to generate gold (Au) ion source and produce high current under applying an electric potential in an argon ambient gas environment. Two Q-switched Nd:YAG lasers operating at 1064 and 266 nm wavelengths are combined in an unconventional orthogonal (crossed-beam) double-pulse configuration with 45° angle to focus on a gold target along with a spectrometer for spectral analysis of gold plasma. The properties of gold plasma produced under double-pulse lasers excitation were studied. The velocity distribution function (VDF) of the emitted plasma was studied using a dedicated Faraday-cup ion probe (FCIP) under argon gas discharge. The experimental parameters were optimized to attain the best signal to noise (S/N) ratio. The results depicted that the VDF and current signals depend on the discharge applied voltage, laser intensity, laser wavelength and ambient argon gas pressure. A seven-fold increases in the current signal by increasing the discharge applied voltage and ion velocity under applying double-pulse lasers field. The plasma parameters (electron temperature and density) were also studied and their dependence on the delay (times between the excitation laser pulse and the opening of camera shutter) was investigated as well. This study could provide significant reference data for the optimization and design of DPLA systems engaged in laser induced plasma deposition thin films and facing components diagnostics.

Plasma Ion Sources for Atmospheric Pressure Ionization Mass Spectrometry.

NASA Astrophysics Data System (ADS)

Zhao, Jian-Guo

1994-01-01

Atmospheric pressure ionization (API) sources using direct-current (DC) and radio-frequency (RF) plasma have been developed in this thesis work. These ion sources can provide stable discharge currents of ~ 1 mA, 2-3 orders of magnitude larger than that of the corona discharge, a widely used API source. The plasmas can be generated and maintained in 1 atm of various buffer gases by applying -500 to -1000 V (DC plasma) or 1-15 W with a frequency of 165 kHz (RF plasma) on the needle electrode. These ion sources have been used with liquid injection to detect various organic compounds of pharmaceutical, biotechnological and environmental interest. Key features of these ion sources include soft ionization with the protonated molecule as the largest peak, and superb sensitivity with detection limits in the low picogram or femtomole range and a linear dynamic range over ~4 orders of magnitude. The RF plasma has advantages over the DC plasma in its ability to operate in various buffer gases and to produce a more stable plasma. Factors influencing the performance of the ion sources have been studied, including RF power level, liquid flow rate, chamber temperature, solvent composition, and voltage affecting the collision induced dissociation (CID). Ionization of hydrocarbons by the RF plasma API source was also studied. Soft ionization is generally produced. To obtain high sensitivity, the ion source must be very dry and the needle-to-orifice distance must be small. Nitric oxide was used to enhance the sensitivity. The RF plasma source was then used for the analysis of hydrocarbons in auto emissions. Comparisons between the corona discharge and the RF plasma have been made in terms of discharge current, ion residence time, and the ion source model. The RF plasma source provides larger linear dynamic range and higher sensitivity than the corona discharge, due to its much larger discharge current. The RF plasma was also observed to provide longer ion residence times and was not limited by space-charge effect as in the corona source.

Effects of hydrocarbon contamination on ozone generation with dielectric barrier discharges

NASA Astrophysics Data System (ADS)

Lopez, Jose L.; Vezzu, Guido; Freilich, Alfred; Paolini, Bernhard

2013-08-01

The increasing usage of the feed gases of lower grade liquid oxygen (LOX) containing higher levels of trace hydrocarbon impurities in dielectric barrier discharge (DBD) for ozone generation requires a better understanding of the kinetics of the by-product formation resulting from reactions involving these hydrocarbon impurities. As a case study of hydrocarbon impurities, the kinetics of CH4 conversion in DBDs and the subsequent HNO3 formation were investigated by means of gas-phase plasma diagnostics, supported by detailed process modeling, and extensive in-situ and ex-situ by-product analysis. The by-products formation in the plasma with the presence of CH4, were found to differ significantly in oxygen-fed generators as compared to generators fed with oxygen/nitrogen mixtures. The amount of HNO3 formed depends on the concentration of NOx formed in the plasma and the amount of CH4 that is converted, but not on the O3 concentration. In the present work we have investigated CH4 concentrations of up to 1.95 wt% of the feed gas. The rate of deterioration of the overall ozone generator performance was found to be affected by the concentration of nitrogen in the oxygen/nitrogen mixture.

CO2 Dissociation by Low Current Gliding Discharge in the Reverse Vortex Flow

NASA Astrophysics Data System (ADS)

Gutsol, Alexander

2012-10-01

If performed with high energy efficiency, plasma-chemical dissociation of carbon dioxide can be a way of converting and storing energy when there is an excess of electric energy, for example generated by solar elements of wind turbines. CO2 dissociation with efficiency of up to 90% was reported earlier for low pressure microwave discharge in supersonic flow. A new plasma-chemical system uses a low current gliding discharge in the reverse vortex flow of plasma gas. The system is a development of the Gliding Arc in Tornado reactor. The system was used to study dissociation of CO2 in wide ranges of the following experimental parameters: reactor pressure (15-150 kPa), discharge current (50-500 mA), gas flow rate (3-30 liters per minute), and electrode gap length (1-10 cm). Additionally, the effect of thermal energy recuperation on CO2 dissociation efficiency was tested. Plasma chemical efficiency of CO2 dissociation is very low (about 3%) in a short discharge at low pressures (about 15 kPa) when it is defined by electronic excitation. The highest efficiency (above 40%) was reached at pressures 50-70 kPa in a long discharge with thermal energy recuperation. It means that the process is controlled by thermal dissociation with subsequent effective quenching. Plasma chemical efficiency was determined from the data of chromatographic analysis and oscilloscope electric power integration, and also was checked calorimetrically by the thermal balance of the system.

Dose-current discharge correlation analysis in a Mather type Plasma Focus device for medical applications

NASA Astrophysics Data System (ADS)

Sumini, M.; Mostacci, D.; Tartari, A.; Mazza, A.; Cucchi, G.; Isolan, L.; Buontempo, F.; Zironi, I.; Castellani, G.

2017-11-01

In a Plasma Focus device the plasma collapses into the pinch where it reaches thermonuclear conditions for a few tens of nanoseconds, becoming a multi-radiation source. The nature of the radiation generated depends on the gas filling the chamber and the device working parameters. The self-collimated electron beam generated in the backward direction with respect to the plasma motion is one of the main radiation sources of interest also for medical applications. The electron beam may be guided against a high Z material target to produce an X-ray beam. This technique offers an ultra-high dose rate source of X-rays, able to deliver during the pinch a massive dose (up to 1 Gy per discharge for the PFMA-3 test device), as measured with EBT3 GafchromicⒸfilm tissue equivalent dosimeters. Given the stochastic behavior of the discharge process, a reliable on-line estimate of the dose-delivered is a very challenging task, in some way preventing a systematic application as a potentially interesting therapy device. This work presents an approach to linking the dose registered by the EBT3 GafchromicⒸfilms with the information contained in the signal recorded during the current discharge process. Processing the signal with the Wigner-Ville distribution, a spectrogram was obtained, displaying the information on intensity at various frequency scales, identifying the band of frequencies representative of the pinch events and define some patterns correlated with the dose.

Synthesis and investigation of reaction mechanisms of diamondoids obtained by dielectric barrier discharge microplasma reactors operated in adamantane - argon - methane - hydrogen mixtures at atmospheric pressure

NASA Astrophysics Data System (ADS)

Stauss, Sven; Ishii, Chikako; Pai, David Z.; Terashima, Kazuo

2013-09-01

Diamondoids, sp3 hybridized molecules consisting of a cage-like carbon framework with hydrogen terminations, hold promise for many applications: biotechnology, medicine, and opto- and nanoelectronics. So far, diamondoids consisting of more than four cage units have been synthesized by electric discharge and pulsed laser plasmas in supercritical fluids, but the generation of plasmas in high-pressure media is not straightforward. Here we present an alternative, continuous flow process, where diamondoids are synthesized by dielectric barrier discharges inside microreactors. The plasmas were generated at peak-to-peak voltages of 3 - 4 kV at a frequency of 10 kHz, in Ar (96 - 100%-vol) - methane (0 - 4%-vol) - hydrogen (0 - 4%-vol) mixtures, at atmospheric pressure and flow rates of 2 - 20 sccm. As a precursor we used the first diamondoid, adamantane, whose density was controlled by adjusting the reactor temperature in the range from 293 to 323 K. Gas chromatography - mass spectrometry analysis indicated the synthesis of the second diamondoid, diamantane, and the presence of alkylated adamantane derivatives suggests a stepwise reaction mechanism. We will also discuss the influence of the plasma gas composition and precursor density on the diamondoid synthesis. Grant No. 21110002, MEXT, Japan.

Regulation characteristics of oxide generation and formaldehyde removal by using volume DBD reactor

NASA Astrophysics Data System (ADS)

Bingyan, CHEN; Xiangxiang, GAO; Ke, CHEN; Changyu, LIU; Qinshu, LI; Wei, SU; Yongfeng, JIANG; Xiang, HE; Changping, ZHU; Juntao, FEI

2018-02-01

Discharge plasmas in air can be accompanied by ultraviolet (UV) radiation and electron impact, which can produce large numbers of reactive species such as hydroxyl radical (OH·), oxygen radical (O·), ozone (O3), and nitrogen oxides (NO x ), etc. The composition and dosage of reactive species usually play an important role in the case of volatile organic compounds (VOCs) treatment with the discharge plasmas. In this paper, we propose a volume discharge setup used to purify formaldehyde in air, which is configured by a plate-to-plate dielectric barrier discharge (DBD) channel and excited by an AC high voltage source. The results show that the relative spectral-intensity from DBD cell without formaldehyde is stronger than the case with formaldehyde. The energy efficiency ratios (EERs) of both oxides yield and formaldehyde removal can be regulated by the gas flow velocity in DBD channel, and the most desirable processing effect is the gas flow velocity within the range from 2.50 to 3.33 m s-1. Moreover, the EERs of both the generated dosages of oxides (O3 and NO2) and the amount of removed formaldehyde can also be regulated by both of the applied voltage and power density loaded on the DBD cell. Additionally, the EERs of both oxides generation and formaldehyde removal present as a function of normal distribution with increasing the applied power density, and the peak of the function is appeared in the range from 273.5 to 400.0 W l-1. This work clearly demonstrates the regulation characteristic of both the formaldehyde removal and oxides yield by using volume DBD, and it is helpful in the applications of VOCs removal by using discharge plasma.

Nanoelectronics and Plasma Processing---The Next 15 Years and Beyond

NASA Astrophysics Data System (ADS)

Lieberman, Michael A.

2006-10-01

The number of transistors per chip has doubled every 2 years since 1959, and this doubling will continue over the next 15 years as transistor sizes shrink. There has been a 25 million-fold decrease in cost for the same performance, and in 15 years a desktop computer will be hundreds of times more powerful than one today. Transistors now have 37 nm (120 atoms) gate lengths and 1.5 nm (5 atoms) gate oxide thicknesses. The smallest working transistor has a 5 nm (17 atoms) gate length, close to the limiting gate length, from simulations, of about 4 nm. Plasma discharges are used to fabricate hundreds of billions of these nano-size transistors on a silicon wafer. These discharges have evolved from a first generation of ``low density'' reactors capacitively driven by a single source, to a second generation of ``high density'' reactors (inductive and electron cyclotron resonance) having two rf power sources, in order to control independently the ion flux and ion bombarding energy to the substrate. A third generation of ``moderate density'' reactors, driven capacitively by one high and one low frequency rf source, is now widely used. Recently, triple frequency and combined dc/dual frequency discharges have been investigated, to further control processing characteristics, such as ion energy distributions, uniformity, and plasma etch selectivities. There are many interesting physics issues associated with these discharges, including stochastic heating of discharge electrons by dual frequency sheaths, nonlinear frequency interactions, powers supplied by the multi-frequency sources, and electromagnetic effects such as standing waves and skin effects. Beyond the 4 nm transistor limit lies a decade of further performance improvements for conventional nanoelectronics, and beyond that, a dimly-seen future of spintronics, single-electron transistors, cross-bar latches, and molecular electronics.

D-D neutron generator development at LBNL.

PubMed

Reijonen, J; Gicquel, F; Hahto, S K; King, M; Lou, T-P; Leung, K-N

2005-01-01

The plasma and ion source technology group in Lawrence Berkeley National Laboratory is developing advanced, next generation D-D neutron generators. There are three distinctive developments, which are discussed in this presentation, namely, multi-stage, accelerator-based axial neutron generator, high-output co-axial neutron generator and point source neutron generator. These generators employ RF-induction discharge to produce deuterium ions. The distinctive feature of RF-discharge is its capability to generate high atomic hydrogen species, high current densities and stable and long-life operation. The axial neutron generator is designed for applications that require fast pulsing together with medium to high D-D neutron output. The co-axial neutron generator is aimed for high neutron output with cw or pulsed operation, using either the D-D or D-T fusion reaction. The point source neutron generator is a new concept, utilizing a toroidal-shaped plasma generator. The beam is extracted from multiple apertures and focus to the target tube, which is located at the middle of the generator. This will generate a point source of D-D, T-T or D-T neutrons with high output flux. The latest development together with measured data will be discussed in this article.

Computational and experimental investigation of plasma deflagration jets and detonation shocks in coaxial plasma accelerators

NASA Astrophysics Data System (ADS)

Subramaniam, Vivek; Underwood, Thomas C.; Raja, Laxminarayan L.; Cappelli, Mark A.

2018-02-01

We present a magnetohydrodynamic (MHD) numerical simulation to study the physical mechanisms underlying plasma acceleration in a coaxial plasma gun. Coaxial plasma accelerators are known to exhibit two distinct modes of operation depending on the delay between gas loading and capacitor discharging. Shorter delays lead to a high velocity plasma deflagration jet and longer delays produce detonation shocks. During a single operational cycle that typically consists of two discharge events, the plasma acceleration exhibits a behavior characterized by a mode transition from deflagration to detonation. The first of the discharge events, a deflagration that occurs when the discharge expands into an initially evacuated domain, requires a modification of the standard MHD algorithm to account for rarefied regions of the simulation domain. The conventional approach of using a low background density gas to mimic the vacuum background results in the formation of an artificial shock, inconsistent with the physics of free expansion. To this end, we present a plasma-vacuum interface tracking framework with the objective of predicting a physically consistent free expansion, devoid of the spurious shock obtained with the low background density approach. The interface tracking formulation is integrated within the MHD framework to simulate the plasma deflagration and the second discharge event, a plasma detonation, formed due to its initiation in a background prefilled with gas remnant from the deflagration. The mode transition behavior obtained in the simulations is qualitatively compared to that observed in the experiments using high framing rate Schlieren videography. The deflagration mode is further investigated to understand the jet formation process and the axial velocities obtained are compared against experimentally obtained deflagration plasma front velocities. The simulations are also used to provide insight into the conditions responsible for the generation and sustenance of the magnetic pinch. The pinch width and number density distribution are compared to experimentally obtained data to calibrate the inlet boundary conditions used to set up the plasma acceleration problem.

High-order harmonic generation in a capillary discharge

DOEpatents

Rocca, Jorge J.; Kapteyn, Henry C.; Mumane, Margaret M.; Gaudiosi, David; Grisham, Michael E.; Popmintchev, Tenio V.; Reagan, Brendan A.

2010-06-01

A pre-ionized medium created by a capillary discharge results in more efficient use of laser energy in high-order harmonic generation (HHG) from ions. It extends the cutoff photon energy, and reduces the distortion of the laser pulse as it propagates down the waveguide. The observed enhancements result from a combination of reduced ionization energy loss and reduced ionization-induced defocusing of the driving laser as well as waveguiding of the driving laser pulse. The discharge plasma also provides a means to spectrally tune the harmonics by tailoring the initial level of ionization of the medium.

On the Asymmetric Focusing of Low-Emittance Electron Bunches via Active Lensing by Using Capillary Discharges

NASA Astrophysics Data System (ADS)

Bulanov, Stepan; Bagdasarov, Gennadiy; Bobrova, Nadezhda; Boldarev, Alexey; Olkhovskaya, Olga; Sasorov, Pavel; Gasilov, Vladimir; Barber, Samuel; Gonsalves, Anthony; Schroeder, Carl; van Tilborg, Jeroen; Esarey, Eric; Leemans, Wim; Levato, Tadzio; Margarone, Daniele; Korn, Georg; Kando, Masaki; Bulanov, Sergei

2017-10-01

A novel method for asymmetric focusing of electron beams is proposed. The scheme is based on the active lensing technique, which takes advantage of the strong inhomogeneous magnetic field generated inside the capillary discharge plasma to focus the ultrarelativistic electrons. The plasma and magnetic field parameters inside a capillary discharge are described theoretically and modeled with dissipative MHD simulations to enable analysis of capillaries of oblong rectangle cross-sections implying that large aspect ratio rectangular capillaries can be used to form flat electron bunches. The effect of the capillary cross-section on the electron beam focusing properties were studied using the analytical methods and simulation- derived magnetic field map showing the range of the capillary discharge parameters required for producing the high quality flat electron beams.

Research on Plasma Synthetic Jet Actuator

NASA Astrophysics Data System (ADS)

Che, X. K.; Nie, W. S.; Hou, Z. Y.

2011-09-01

Circular dielectric barrier surface discharge (DBDs) actuator is a new concept of zero mass synthetic jet actuator. The characteristic of discharge and flow control effect of annular-circular plasma synthetic jet actuator has been studied by means of of numerical simulation and experiment. The discharge current density, electron density, electrostatic body force density and flowfield have been obtained. The results show annular-circular actuator can produce normal jet whose velocity will be greater than 2.0 m/s. The jet will excite circumfluence. In order to insure the discharge is generated in the exposed electrode annular and produce centripetal and normal electrostatic body force, the width and annular diameter of exposed electrode must be big enough, or an opposite phase drove voltage potential should be applied between the two electrodes.

Characteristic properties of the frame-antenna-produced RF discharge evolution in the Uragan-3M torsatron

NASA Astrophysics Data System (ADS)

Chechkin, V. V.; Grigor'eva, L. I.; Pavlichenko, R. O.; Kulaga, A. Ye.; Zamanov, N. V.; Moiseenko, V. E.; Burchenko, P. Ya.; Lozin, A. V.; Tsybenko, S. A.; Tarasov, I. K.; Pankratov, I. M.; Grekov, D. L.; Beletskii, A. A.; Kasilov, A. A.; Voitsenya, V. S.; Pashnev, V. K.; Konovalov, V. G.; Shapoval, A. N.; Mironov, Yu. K.; Romanov, V. S.

2014-08-01

In the ℓ = 3 Uragan-3M torsatron, hydrogen plasma is produced and heated by RF fields in the Alfvén range of frequencies (ω ≲ ω ci ). To this end, a frame antenna with a broad spectrum of generated parallel wavenumbers is used. The RF discharge evolution is studied experimentally at different values of the RF power fed to the antenna (the anode voltage of the oscillator and the antenna current) and the initial pressure of the fueling gas. It is shown that, depending on the antenna current and hydrogen pressure, the discharge can operate in two regimes differing in the plasma density, temperature, and particle loss. The change in the discharge regime with increasing anode voltage is steplike in character. The particular values of the anode voltage and pressure at which the change occurs are affected by RF preionization or breakdown stabilization by a microwave discharge. The obtained results will be used in future experiments to choose the optimal regimes of the frame-antenna-produced RF discharge as a target for the production and heating of a denser plasma by another, shorter wavelength three-half-turn antenna.

Spectroscopic diagnosis of plasma in atmospheric pressure negative pulsed gas-liquid discharge with nozzle-cylinder electrode

NASA Astrophysics Data System (ADS)

Ming, SUN; Zhan, TAO; Zhipeng, ZHU; Dong, WANG; Wenjun, PAN

2018-05-01

The plasma characteristics of a gas-liquid phase discharge reactor were investigated by optical and electrical methods. The nozzle-cylinder electrode in the discharge reactor was supplied with a negative nanosecond pulsed generator. The optical emission spectrum diagnosis revealed that OH (A2∑+ → X2Π, 306–309 nm), N2 (C3Π→B3Πg, 337 nm), O (3p5p→3s5s0, 777.2 nm) and O (3p3p→3s3s0, 844.6 nm) were produced in the discharge plasma channels. The electron temperature (T e) was calculated from the emission relative intensity ratio between the atomic O 777.2 nm and 844.6 nm, and it increased with the applied voltage and the pulsed frequency and fell within the range of 0.5–0.8 eV. The gas temperature (T g) that was measured by Lifbase was in a range from 400 K to 600 K.

Development of alternative plasma sources for cavity ring-down measurements of mercury.

PubMed

Duan, Yixiang; Wang, Chuji; Scherrer, Susan T; Winstead, Christopher B

2005-08-01

We have been exploring innovative technologies for elemental and hyperfine structure measurements using cavity ring-down spectroscopy (CRDS) combined with various plasma sources. A laboratory CRDS system utilizing a tunable dye laser is employed in this work to demonstrate the feasibility of the technology. An in-house fabricated sampling system is used to generate aerosols from solution samples and introduce the aerosols into the plasma source. The ring-down signals are monitored using a photomultiplier tube and recorded using a digital oscilloscope interfaced to a computer. Several microwave plasma discharge devices are tested for mercury CRDS measurement. Various discharge tubes have been designed and tested to reduce background interference and increase the sample path length while still controlling turbulence generated from the plasma gas flow. Significant background reduction has been achieved with the implementation of the newly designed tube-shaped plasma devices, which has resulted in a detection limit of 0.4 ng/mL for mercury with the plasma source CRDS. The calibration curves obtained in this work readily show that linearity over 2 orders of magnitude can be obtained with plasma-CRDS for mercury detection. In this work, the hyperfine structure of mercury at the experimental plasma temperatures is clearly identified. We expect that plasma source cavity ring-down spectroscopy will provide enhanced capabilities for elemental and isotopic measurements.

Study on re-sputtering during CN{sub x} film deposition through spectroscopic diagnostics of plasma

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liang, Peipei; Yang, Xu; Li, Hui

2015-10-15

A nitrogen-carbon plasma was generated during the deposition of carbon nitride (CN{sub x}) thin films by pulsed laser ablation of a graphite target in a discharge nitrogen plasma, and the optical emission of the generated nitrogen-carbon plasma was measured for the diagnostics of the plasma and the characterization of the process of CN{sub x} film deposition. The nitrogen-carbon plasma was recognized to contain various species including nitrogen molecules and molecular ions excited in the ambient N{sub 2} gas, carbon atoms and atomic ions ablated from the graphite target and CN radicals. The temporal evolution and spatial distribution of the CNmore » emission and their dependence on the substrate bias voltage show two groups of CN radicals flying in opposite directions. One represents the CN radicals formed as the products of the reactions occurring in the nitrogen-carbon plasma, revealing the reactive deposition of CN{sub x} film due to the reactive expansion of the ablation carbon plasma in the discharge nitrogen plasma and the effective formation of gaseous CN radicals as precursors for CN{sub x} film growth. The other one represents the CN radicals re-sputtered from the growing CN{sub x} film by energetic plasma species, evidencing the re-sputtering of the growing film accompanying film growth. And, the re-sputtering presents ion-induced sputtering features.« less

Development of fully non-inductive plasmas heated by medium and high-harmonic fast waves in the national spherical torus experiment upgrade

NASA Astrophysics Data System (ADS)

Taylor, G.; Poli, F.; Bertelli, N.; Harvey, R. W.; Hosea, J. C.; Mueller, D.; Perkins, R. J.; Phillips, C. K.; Raman, R.

2015-12-01

A major challenge for spherical tokamak development is to start-up and ramp-up the plasma current (Ip) without using a central solenoid. Experiments in the National Spherical Torus eXperiment (NSTX) demonstrated that 1.4 MW of 30 MHz high-harmonic fast wave (HHFW) power could generate an Ip = 300 kA H-mode discharge with a non-inductive Ip fraction, fNI ˜ 0.7. The discharge had an axial toroidal magnetic field (BT(0)) of 0.55 T, the maximum BT(0) available on NSTX. NSTX has undergone a major upgrade (NSTX-U), that will eventually allow the generation of BT(0) ≤ 1 T and Ip ≤ 2 MA plasmas. Full wave simulations of 30 MHz HHFW and medium harmonic fast wave (MHFW) heating in NSTX-U predict significantly reduced FW power loss in the plasma edge at the higher BT(0) achievable in NSTX-U. HHFW experiments will aim to generate stable, fNI ˜ 1, Ip = 300 kA H-mode plasmas and to ramp Ip from 250 to 400 kA with FW power. Time-dependent TRANSP simulations are used to develop non-inductive Ip ramp-up and sustainment using 30 MHz FW power. This paper presents results from these RF simulations and plans for developing non-inductive plasmas heated by FW power.

Dwell time considerations for large area cold plasma decontamination

NASA Astrophysics Data System (ADS)

Konesky, Gregory

2009-05-01

Atmospheric discharge cold plasmas have been shown to be effective in the reduction of pathogenic bacteria and spores and in the decontamination of simulated chemical warfare agents, without the generation of toxic or harmful by-products. Cold plasmas may also be useful in assisting cleanup of radiological "dirty bombs." For practical applications in realistic scenarios, the plasma applicator must have both a large area of coverage, and a reasonably short dwell time. However, the literature contains a wide range of reported dwell times, from a few seconds to several minutes, needed to achieve a given level of reduction. This is largely due to different experimental conditions, and especially, different methods of generating the decontaminating plasma. We consider these different approaches and attempt to draw equivalencies among them, and use this to develop requirements for a practical, field-deployable plasma decontamination system. A plasma applicator with 12 square inches area and integral high voltage, high frequency generator is described.

Electric field measurements in a near atmospheric pressure nanosecond pulse discharge with picosecond electric field induced second harmonic generation

NASA Astrophysics Data System (ADS)

Goldberg, Benjamin M.; Chng, Tat Loon; Dogariu, Arthur; Miles, Richard B.

2018-02-01

We present an optical electric field measurement method for use in high pressure plasma discharges. The method is based upon the field induced second harmonic generation technique and can be used for localized electric field measurements with sub-nanosecond resolution in any gaseous species. When an external electric field is present, a dipole is induced in the typically centrosymmetric medium, allowing for second harmonic generation with signal intensities which scale by the square of the electric field. Calibrations have been carried out in 100 Torr room air, and a minimum sensitivity of 450 V/cm is demonstrated. Measurements were performed with nanosecond or faster temporal resolution in a 100 Torr room air environment both with and without a plasma present. It was shown that with no plasma present, the field follows the applied voltage to gap ratio, as measured using the back current shunt method. When the electric field is strong enough to exceed the breakdown threshold, the measured field was shown to exceed the anticipated voltage to gap ratio which is taken as an indication of the ionization wave front as it sweeps through the plasma volume.

Performance Characterization of a Novel Plasma Thruster to Provide a Revolutionary Operationally Responsive Space Capability with Micro- and Nano-Satellites

DTIC Science & Technology

2011-03-24

and radiation resistance of rare earth permanent magnets for applications such as ion thrusters and high efficiency Stirling Radioisotope Generators...from Electron Transitioning Discharge Current Discharge Power Discharge Voltage Θ Divergence Angle Earths Gravity at Sea Level...Hall effect thruster HIVAC High Voltage Hall Accelerator LEO Low Earth Orbit LDS Laser Displacement System LVDT Linear variable differential

Honeycomblike large area LaB6 plasma source for Multi-Purpose Plasma facility

NASA Astrophysics Data System (ADS)

Woo, Hyun-Jong; Chung, Kyu-Sun; You, Hyun-Jong; Lee, Myoung-Jae; Lho, Taihyeop; Choh, Kwon Kook; Yoon, Jung-Sik; Jung, Yong Ho; Lee, Bongju; Yoo, Suk Jae; Kwon, Myeon

2007-10-01

A Multi-Purpose Plasma (MP2) facility has been renovated from Hanbit mirror device [Kwon et al., Nucl. Fusion 43, 686 (2003)] by adopting the same philosophy of diversified plasma simulator (DiPS) [Chung et al., Contrib. Plasma Phys. 46, 354 (2006)] by installing two plasma sources: LaB6 (dc) and helicon (rf) plasma sources; and making three distinct simulators: divertor plasma simulator, space propulsion simulator, and astrophysics simulator. During the first renovation stage, a honeycomblike large area LaB6 (HLA-LaB6) cathode was developed for the divertor plasma simulator to improve the resistance against the thermal shock fragility for large and high density plasma generation. A HLA-LaB6 cathode is composed of the one inner cathode with 4in. diameter and the six outer cathodes with 2in. diameter along with separate graphite heaters. The first plasma is generated with Ar gas and its properties are measured by the electric probes with various discharge currents and magnetic field configurations. Plasma density at the middle of central cell reaches up to 2.6×1012 cm-3, while the electron temperature remains around 3-3.5eV at the low discharge current of less than 45A, and the magnetic field intensity of 870G. Unique features of electric property of heaters, plasma density profiles, is explained comparing with those of single LaB6 cathode with 4in. diameter in DiPS.

Honeycomblike large area LaB6 plasma source for Multi-Purpose Plasma facility.

PubMed

Woo, Hyun-Jong; Chung, Kyu-Sun; You, Hyun-Jong; Lee, Myoung-Jae; Lho, Taihyeop; Choh, Kwon Kook; Yoon, Jung-Sik; Jung, Yong Ho; Lee, Bongju; Yoo, Suk Jae; Kwon, Myeon

2007-10-01

A Multi-Purpose Plasma (MP(2)) facility has been renovated from Hanbit mirror device [Kwon et al., Nucl. Fusion 43, 686 (2003)] by adopting the same philosophy of diversified plasma simulator (DiPS) [Chung et al., Contrib. Plasma Phys. 46, 354 (2006)] by installing two plasma sources: LaB(6) (dc) and helicon (rf) plasma sources; and making three distinct simulators: divertor plasma simulator, space propulsion simulator, and astrophysics simulator. During the first renovation stage, a honeycomblike large area LaB(6) (HLA-LaB(6)) cathode was developed for the divertor plasma simulator to improve the resistance against the thermal shock fragility for large and high density plasma generation. A HLA-LaB(6) cathode is composed of the one inner cathode with 4 in. diameter and the six outer cathodes with 2 in. diameter along with separate graphite heaters. The first plasma is generated with Ar gas and its properties are measured by the electric probes with various discharge currents and magnetic field configurations. Plasma density at the middle of central cell reaches up to 2.6 x 10(12) cm(-3), while the electron temperature remains around 3-3.5 eV at the low discharge current of less than 45 A, and the magnetic field intensity of 870 G. Unique features of electric property of heaters, plasma density profiles, is explained comparing with those of single LaB(6) cathode with 4 in. diameter in DiPS.

Physical investigation of a quad confinement plasma source

NASA Astrophysics Data System (ADS)

Knoll, Aaron; Lucca Fabris, Andrea; Young, Christopher; Cappelli, Mark

2016-10-01

Quad magnetic confinement plasma sources are novel magnetized DC discharges suitable for applications in a broad range of fields, particularly space propulsion, plasma etching and deposition. These sources contain a square discharge channel with magnetic cusps at the four lateral walls, enhancing plasma confinement and electron residence time inside the device. The magnetic field topology is manipulated using four independent electromagnets on each edge of the channel, tuning the properties of the generated plasma. We characterize the plasma ejected from the quad confinement sources using a combination of traditional electrostatic probes and non-intrusive laser-based diagnostics. Measurements show a strong ion acceleration layer located 8 cm downstream of the exit plane, beyond the extent of the magnetic field. The ion velocity field is investigated with different magnetic configurations, demonstrating how ion trajectories may be manipulated. C.Y. acknowledges support from the DOE NSSA Stewardship Science Graduate Fellowship under contract DE-FC52-08NA28752.

Stable aqueous dispersions of functionalized multi-layer graphene by pulsed underwater plasma exfoliation of graphite

NASA Astrophysics Data System (ADS)

Meyer-Plath, Asmus; Beckert, Fabian; Tölle, Folke J.; Sturm, Heinz; Mülhaupt, Rolf

2016-02-01

A process was developed for graphite particle exfoliation in water to stably dispersed multi-layer graphene. It uses electrohydraulic shockwaves and the functionalizing effect of solution plasma discharges in water. The discharges were excited by 100 ns high voltage pulsing of graphite particle chains that bridge an electrode gap. The underwater discharges allow simultaneous exfoliation and chemical functionalization of graphite particles to partially oxidized multi-layer graphene. Exfoliation is caused by shockwaves that result from rapid evaporation of carbon and water to plasma-excited gas species. Depending on discharge energy and locus of ignition, the shockwaves cause stirring, erosion, exfoliation and/or expansion of graphite flakes. The process was optimized to produce long-term stable aqueous dispersions of multi-layer graphene from graphite in a single process step without requiring addition of intercalants, surfactants, binders or special solvents. A setup was developed that allows continuous production of aqueous dispersions of flake size-selected multi-layer graphenes. Due to the well-preserved sp2-carbon structure, thin films made from the dispersed graphene exhibited high electrical conductivity. Underwater plasma discharge processing exhibits high innovation potential for morphological and chemical modifications of carbonaceous materials and surfaces, especially for the generation of stable dispersions of two-dimensional, layered materials.

Killing Microorganisms with the One Atmosphere Uniform Glow Discharge Plasma

NASA Astrophysics Data System (ADS)

South, Suzanne; Kelly-Wintenberg, Kimberly; Montie, T. C.; Reece Roth, J.; Sherman, Daniel; Morrison, Jim; Chen, Zhiyu; Karakaya, Fuat

2000-10-01

There is an urgent need for the development of new technologies for sterilization and decontamination in the fields of healthcare and industrial and food processing that are safe, cost-effective, broad-spectrum, and not deleterious to samples. One technology that meets these criteria is the One Atmosphere Uniform Glow Discharge Plasma (OAUGDP). The OAUGDP operates in air and produces uniform plasma without filamentary discharges at room temperature, making this technology advantageous for sterilization of heat sensitive materials. The OAUGDP operates in a frequency band determined by the ion trapping mechanisms provided that, for air, the electric field is above 8.5kV/cm. The OAUGDP efficiently generates plasma reactive oxygen species (ROS) including atomic oxygen and oxygen free radicals without the requirement of a vacuum system. We have demonstrated the efficacy of the OAUGDP in killing microorganisms including bacteria, yeast, viruses, and spores in seconds to minutes on a variety of surfaces such as glass, films and fabrics, stainless steel, paper, and agar.

Direct coupling of pulsed radio frequency and pulsed high power in novel pulsed power system for plasma immersion ion implantation.

PubMed

Gong, Chunzhi; Tian, Xiubo; Yang, Shiqin; Fu, Ricky K Y; Chu, Paul K

2008-04-01

A novel power supply system that directly couples pulsed high voltage (HV) pulses and pulsed 13.56 MHz radio frequency (rf) has been developed for plasma processes. In this system, the sample holder is connected to both the rf generator and HV modulator. The coupling circuit in the hybrid system is composed of individual matching units, low pass filters, and voltage clamping units. This ensures the safe operation of the rf system even when the HV is on. The PSPICE software is utilized to optimize the design of circuits. The system can be operated in two modes. The pulsed rf discharge may serve as either the seed plasma source for glow discharge or high-density plasma source for plasma immersion ion implantation (PIII). The pulsed high-voltage glow discharge is induced when a rf pulse with a short duration or a larger time interval between the rf and HV pulses is used. Conventional PIII can also be achieved. Experiments conducted on the new system confirm steady and safe operation.

Potential Industrial Applications of the One Atmosphere Uniform Glow Discharge Plasma (OAUGDP) Operating in Ambient Air

NASA Astrophysics Data System (ADS)

Reece Roth, J.

2004-11-01

The majority of industrial plasma processing with glow discharges has been conducted at pressures below 10 torr. This tends to limit applications to high value workpieces as a result of the high capital cost of vacuum systems and the production constraints of batch processing. It has long been recognized that glow discharge plasmas would play a much larger industrial role if they could be generated at one atmosphere. The One Atmosphere Uniform Glow Discharge Plasma (OAUGDP), developed at the University of Tennessee's Plasma Sciences Laboratory, is a non-thermal RF plasma operating on displacement currents with the time-resolved characteristics of a classical low pressure DC normal glow discharge. As a glow discharge, the OAUGDP operates with maximum electrical efficiency at the Stoletow point, where the energy input per ion-electron pair is a minimum [1, 2]. Several interdisciplinary teams have investigated potential applications of the OAUGDP. These teams included collaborators from the UTK Textiles and Nonwovens Development Center (TANDEC), and the Departments of Electrical and Computer Engineering, Microbiology, and Food Science and Technology, as well as the NASA Langley Research Center. The potential applications of the OAUGDP have all been at one atmosphere and room temperature, using air as the working gas. These applications include sterilizing medical and dental equipment; sterilizable air filters to deal with the "sick building syndrome"; removal of soot from Diesel engine exhaust; subsonic plasma aerodynamic effects, including flow re-attachment to airfoils and boundary layer modification; electrohydrodynamic (EDH) flow control of working gases; increasing the surface energy of materials; improving the adhesion of paints and electroplated layers: improving the wettability and wickability of fabrics; stripping of photoresist; and plasma deposition and directional etching of potential microelectronic relevance. [1] J. R. Roth, Industrial Plasma Engineering: Volume I, Principles. Institute of Physics Publishing, Bristol and Philadelphia 1995, ISBN 0-7503-0318-2. [2] Roth, J. R. Industrial Plasma Engineering: Volume II Applications to Nonthermal Plasma Processing Institute of Physics Publishing, Bristol and Philadelphia. 2001, ISBN 0-7503-0545-2.

The physics of pulsed streamer discharge in high pressure air and applications to engine techonologies

NASA Astrophysics Data System (ADS)

Lin, Yung-Hsu

The goal of this dissertation is to study high pressure streamers in air and apply it to diesel engine technologies. Nanosecond scale pulsed high voltage discharges in air/fuel mixtures can generate radicals which in turn have been shown to improve combustion efficiency in gasoline fueled internal combustion engines. We are exploring the possibility to extend such transient plasma generation and expected radical species generation to the range of pressures encountered in compression-ignition (diesel) engines having compression ratios of ˜20:1, thereby improving lean burning efficiency and extending the range of lean combustion. At the beginning of this dissertation, research into streamer discharges is reviewed. Then, we conducted experiments of streamer propagation at high pressures, calculated the streamer velocity based on both optical and electrical measurements, and the similarity law was checked by analyzing the streamer velocity as a function of the reduced electric field, E/P. Our results showed that the similarity law is invalid, and an empirical scaling factor, E/√P, is obtained and verified by dimensional analysis. The equation derived from the dimensional analysis will be beneficial to proper electrode and pulse generator design for transient plasma assisted internal engine experiments. Along with the high pressure study, we applied such technique on diesel engine to improve the fuel efficiency and exhaust treatment. We observed a small effect of transient plasma on peak pressure, which implied that transient plasma has the capability to improve the fuel consumption. In addition, the NO can be reduced effectively by the same technique and the energy cost is 30 eV per NO molecule.

Direct current plasma jet at atmospheric pressure operating in nitrogen and air

NASA Astrophysics Data System (ADS)

Deng, X. L.; Nikiforov, A. Yu.; Vanraes, P.; Leys, Ch.

2013-01-01

An atmospheric pressure direct current (DC) plasma jet is investigated in N2 and dry air in terms of plasma properties and generation of active species in the active zone and the afterglow. The influence of working gases and the discharge current on plasma parameters and afterglow properties are studied. The electrical diagnostics show that discharge can be sustained in two different operating modes, depending on the current range: a self-pulsing regime at low current and a glow regime at high current. The gas temperature and the N2 vibrational temperature in the active zone of the jet and in the afterglow are determined by means of emission spectroscopy, based on fitting spectra of N2 second positive system (C3Π-B3Π) and the Boltzmann plot method, respectively. The spectra and temperature differences between the N2 and the air plasma jet are presented and analyzed. Space-resolved ozone and nitric oxide density measurements are carried out in the afterglow of the jet. The density of ozone, which is formed in the afterglow of nitrogen plasma jet, is quantitatively detected by an ozone monitor. The density of nitric oxide, which is generated only in the air plasma jet, is determined by means of mass-spectroscopy techniques.

Large-Volume Resonant Microwave Discharge for Plasma Cleaning of a CEBAF 5-Cell SRF Cavity

DOE Office of Scientific and Technical Information (OSTI.GOV)

J. Mammosser, S. Ahmed, K. Macha, J. Upadhyay, M. Nikoli, S. Popovi, L. Vuakovi

2012-07-01

We report the preliminary results on plasma generation in a 5-cell CEBAF superconducting radio-frequency (SRF) cavity for the application of cavity interior surface cleaning. CEBAF currently has {approx}300 of these five cell cavities installed in the Jefferson Lab accelerator which are mostly limited by cavity surface contamination. The development of an in-situ cavity surface cleaning method utilizing a resonant microwave discharge could lead to significant CEBAF accelerator performance improvement. This microwave discharge is currently being used for the development of a set of plasma cleaning procedures targeted to the removal of various organic, metal and metal oxide impurities. These contaminantsmore » are responsible for the increase of surface resistance and the reduction of RF performance in installed cavities. The CEBAF five cell cavity volume is {approx} 0.5 m2, which places the discharge in the category of large-volume plasmas. CEBAF cavity has a cylindrical symmetry, but its elliptical shape and transversal power coupling makes it an unusual plasma application, which requires special consideration of microwave breakdown. Our preliminary study includes microwave breakdown and optical spectroscopy, which was used to define the operating pressure range and the rate of removal of organic impurities.« less

Collaborative Research: Atmospheric Pressure Plasma-Biomaterial Surface Interactions - Bridging Understanding of APP Sources to Rational Modification of Biomolecules

DOE Office of Scientific and Technical Information (OSTI.GOV)

Graves, David Barry

The overriding objective of this work is to bridge the gap between understanding of atmospheric pressure plasma (APP) sources and predictive chemical modifications of biomolecules. A key aspect of this problem is to understand what oxidizing species are created in water adjacent to APP jets that would ultimately affect aqueous biomolecules. We report the production of highly oxidative species in solutions exposed to a self-pulsed corona discharge in air. We examine how the properties of the target solution (pH, conductivity) and the discharge power affect the discharge stability and the production of H2O2. Indigo carmine, a common organic dye, ismore » used as an indicator of oxidative strength and in particular, hydroxyl radical (OH•) production. The observed rate of indigo oxidation in contact with the discharge far exceeds that predicted from reactions based on concentrations of species measured in the bulk solution. The generation of H2O2 and the oxidation of indigo carmine indicate a high concentration of highly oxidizing species such as OH• at the plasma-liquid interface. These results indicate that reactions at the air plasma-liquid interface play a dominant role in species oxidation during direct non-equilibrium atmospheric pressure plasma (NE-APP) treatment.« less

Improvement of wheat seed vitality by dielectric barrier discharge plasma treatment.

PubMed

Guo, Qiao; Meng, Yiran; Qu, Guangzhou; Wang, Tiecheng; Yang, Fengning; Liang, Dongli; Hu, Shibin

2018-02-01

Influences of discharge voltage on wheat seed vitality were investigated in a dielectric barrier discharge (DBD) plasma system at atmospheric pressure and temperature. Six different treatments were designed, and their discharge voltages were 0.0, 9.0, 11.0, 13.0, 15.0, and 17.0 kV, respectively. Fifty seeds were exposed to the DBD plasma atmosphere with an air flow rate of 1.5 L min -1 for 4 min in each treatment, and then the DBD plasma-treated seeds were prepared for germination in several Petri dishes. Each treatment was repeated three times. Germination indexes, growth indexes, surface topography, water uptake, permeability, and α-amylase activity were measured. DBD plasma treatment at appropriate energy levels had positive effects on wheat seed germination and seedling growth. The germination potential, germination index, and vigor index significantly increased by 31.4%, 13.9%, and 54.6% after DBD treatment at 11.0 kV, respectively, in comparison to the control. Shoot length, root length, dry weight, and fresh weight also significantly increased after the DBD plasma treatment. The seed coat was softened and cracks were observed, systematization of the protein was strengthened, and amount of free starch grain increased after the DBD plasma treatment. Water uptake, relative electroconductivity, soluble protein, and α-amylase activity of the wheat seed were also significantly improved after the DBD plasma treatment. Roles of active species and ultraviolet radiation generated in the DBD plasma process in wheat seed germination and seedling growth are proposed. Bioelectromagnetics. 39:120-131, 2018. © 2017 Wiley Periodicals, Inc. © 2017 Wiley Periodicals, Inc.

Compact Plasma Accelerator for Micropropulsion Applications

NASA Technical Reports Server (NTRS)

Foster, John E.

2001-01-01

There is a need for a low power, light-weight (compact), high specific impulse electric propulsion device to satisfy mission requirements for microsatellite (1 to 20 kg) class missions. Satisfying these requirements entails addressing the general problem of generating a sufficiently dense plasma within a relatively small volume and then accelerating it. In the work presented here, the feasibility of utilizing a magnetic cusp to generate a dense plasma over small length scales of order 1 mm is investigated. This approach could potentially mitigate scaling issues associated with conventional ion thruster plasma containment schemes. Plume and discharge characteristics were documented using a Faraday probe and a retarding potential analyzer.

Self-consistent discharge growing model of helicon plasma

NASA Astrophysics Data System (ADS)

Isayama, Shogo; Hada, Tohru; Shinohara, Shunjiro; Tanikawa, Takao

2015-11-01

Helicon plasma is a high-density and low-temperature plasma generated by the electromagnetic (Helicon) wave excited in the plasma. It is thought to be useful for various applications including electric thrusters. Physics of helicon plasma production involves such fundamental processes as the wave propagation (dispersion relation), collisional and non-collisional wave damping, plasma heating, ionization/recombination of neutral particles, and modification of the dispersion relation by newly ionized plasma. There remain a number of unsolved physical issues such as, how the Helicon and the TG modes influence the plasma density, electron temperature and their spatial profiles. While the Helicon mode is absorbed in the bulk plasma, the TG mode is mostly absorbed near the edge of the plasma. The local power deposition in the helicon plasma is mostly balanced by collisional loss. This local power balance can give rise to the inhomogeneous electron temperature profile that leads to time evolution of density profile and dispersion relation. In our study, we construct a self-consistent model of the discharge evolution that includes the wave excitation, electron heat transfer, and diffusion of charged particles.

Efficient Ionization Investigation for Flow Control and Energy Extraction

NASA Technical Reports Server (NTRS)

Schneider, Steven J.; Kamhawi, Hani; Blankson, Isaiah M.

2009-01-01

Nonequilibrium ionization of air by nonthermal means is explored for hypersonic vehicle applications. The method selected for evaluation generates a weakly ionized plasma using pulsed nanosecond, high-voltage discharges sustained by a lower dc voltage. These discharges promise to provide a means of energizing and sustaining electrons in the air while maintaining a nearly constant ion/neutral molecule temperature. This paper explores the use of short approx.5 nsec, high-voltage approx.12 to 22 kV, repetitive (40 to 100 kHz) discharges in generating a weakly ionized gas sustained by a 1 kV dc voltage in dry air at pressures from 10 to 80 torr. Demonstrated lifetimes of the sustainer discharge current approx.10 to 25 msec are over three orders of magnitude longer than the 5 nsec pulse that generates the electrons. This life is adequate for many high speed flows, enabling the possibility of exploiting weakly ionized plasma phenomena in flow-fields such as those in hypersonic inlets, combustors, and nozzles. Results to date are obtained in a volume of plasma between electrodes in a bell jar. The buildup and decay of the visible emission from the pulser excited air is photographed on an ICCD camera with nanosecond resolution and the time constants for visible emission decay are observed to be between 10 to 15 nsec decreasing as pressure increases. The application of the sustainer voltage does not change the visible emission decay time constant. Energy consumption as indicated by power output from the power supplies is 194 to 669 W depending on pulse repetition rate.

Performance of a green propellant thruster with discharge plasma

NASA Astrophysics Data System (ADS)

Shindo, Takahiro; Wada, Asato; Maeda, Hiroshi; Watanabe, Hiroki; Takegahara, Haruki

2017-02-01

A discharge plasma was applied to initiate the combustion of a hydroxylammonium nitrate-based propellant as a substitute for the catalysts that are typically employed. The resulting thrust and thrust-to-power ratio during short interval firing tests as well as the chamber pressure with a single pulse discharge were evaluated. A 1.5-s firing test generated a maximum thrust of 322 mN along with a thrust-to-power ratio of 0.95 mN/W. During the single-pulse discharge trials, pulsed discharge capacitor energies of 5.4, 10.8, and 16.4 J were assessed, and the maximum chamber pressure was found to increase as the energy was raised. The maximum chamber pressures varied widely between experimental trials, and a 16.4-J energy value resulted in the highest chamber pressure of over 1 MPaG. The time spans between the pulsed discharge and the peak chamber pressure were in the range of 1-2 ms, representing a chamber pressure increase rate much higher than those obtained with standard catalysts.

Inactivation of Bacteria in Oil Field Injected Water by a Pulsed Plasma Discharge Process

NASA Astrophysics Data System (ADS)

Xin, Qing; Li, Zhongjian; Lei, Lecheng; Yang, Bin

2016-09-01

Pulsed plasma discharge was employed to inactivate bacteria in the injection water for an oil field. The effects of water conductivity and initial concentration of bacteria on elimination efficiency were investigated in the batch and continuous flow modes. It was demonstrated that Fe2+ contained in injection water could enhance the elimination efficiency greatly. The addition of reducing agent glutathione (GSH) indicated that active radicals generated by pulsed plasma discharges played an important role in the inactivation of bacteria. Moreover, it was found that the microbial inactivation process for both batch and continuous flow mode well fitted the model based on the Weibull's survival function. supported by Zhejiang Province Welfare Technology Applied Research Project of China (No. 2014C31137), National Natural Science Foundation of China (Nos. 21436007 and U1462201), and the Fundamental Research Funds for the Central Universities of China (No. 2015QNA4032)

Three distinct modes in a surface micro-discharge in atmospheric pressure He + N{sub 2} mixtures

DOE Office of Scientific and Technical Information (OSTI.GOV)

Li, Dong; Liu, Dingxin, E-mail: liudingxin@mail.xjtu.edu.cn; He, Tongtong

2015-12-15

A surface micro-discharge in atmospheric pressure He + N{sub 2} mixtures is studied in this paper with an emphasis on the discharge modes. With the N{sub 2} admixture increasing from 0.1% to 20%, the discharge evolves from a spatially diffuse mode to a filamentary mode during positive half-cycles of the applied voltage. However during the negative half-cycles, an additional patterned mode emerges between the diffuse and the filamentary modes, which has not been reported before to exist in surface micro-discharges. In the diffuse and patterned modes, the plasmas cover almost the entirety of the mesh area during one cycle after plasma ignitionmore » in all mesh elements, and the discharge power increases linearly with the applied voltage. In contrast, plasma coverage of the mesh area is only partial in the filamentary mode and the plasma is more unstable with the discharge power increasing exponentially with the applied voltage. As the surface micro-discharge evolves through the three modes, the density of excited species changes significantly, for instance, the density of N{sub 2}{sup +}(B) drops by ∼20-fold from [N{sub 2}] = 0.2% to 20%. The N{sub 2}{sup +}(B) is predicted to be generated mainly through successive processes of Penning ionization by helium metastables and electron-impact excitation of N{sub 2}{sup +}(X), the latter is most responsible for the density decrease of N{sub 2}{sup +}(B) because much more N{sub 2}{sup +}(X) is converted to N{sub 4}{sup +}(X) as the increase of N{sub 2} fraction. Also, the electron density and electron temperature decrease with the discharge mode transition.« less

Standard/Handbook for RF Ionization Breakdown Prevention in Spacecraft Components

DTIC Science & Technology

2015-06-19

localized glow discharge of the plasma ( corona ) while RF power is being applied. 8.4.3 RF Performance Changes If a breakdown occurs and damages the...in spacecraft components and systems. Ionization breakdown is a high-energy radio frequency (RF) discharge that can occur when the insulating media...energy can be discharged in a small volume, releasing large amounts of heat, melting local surfaces, and generating debris, all of which will likely

Standard/Handbook for RF Ionization Breakdown Prevention in Spacecraft Components

DTIC Science & Technology

2015-06-19

localized glow discharge of the plasma ( corona ) while RF power is being applied. 8.4.3 RF Performance Changes If a breakdown occurs and damages the part...in spacecraft components and systems. Ionization breakdown is a high-energy radio frequency (RF) discharge that can occur when the insulating media...energy can be discharged in a small volume, releasing large amounts of heat, melting local surfaces, and generating debris, all of which will likely

Modeling of inhomogeneous mixing of plasma species in argon-steam arc discharge

NASA Astrophysics Data System (ADS)

Jeništa, J.; Takana, H.; Uehara, S.; Nishiyama, H.; Bartlová, M.; Aubrecht, V.; Murphy, A. B.

2018-01-01

This paper presents numerical simulation of mixing of argon- and water-plasma species in an argon-steam arc discharge generated in a thermal plasma generator with the combined stabilization of arc by axial gas flow (argon) and water vortex. The diffusion of plasma species itself is described by the combined diffusion coefficients method in which the coefficients describe the diffusion of argon ‘gas,’ with respect to water vapor ‘gas.’ Diffusion processes due to the gradients of mass density, temperature, pressure, and an electric field have been considered in the model. Calculations for currents 150-400 A with 15-22.5 standard liters per minute (slm) of argon reveal inhomogeneous mixing of argon and oxygen-hydrogen species with the argon species prevailing near the arc axis. All the combined diffusion coefficients exhibit highly nonlinear distribution of their values within the discharge, depending on the temperature, pressure, and argon mass fraction of the plasma. The argon diffusion mass flux is driven mainly by the concentration and temperature space gradients. Diffusions due to pressure gradients and due to the electric field are of about 1 order lower. Comparison with our former calculations based on the homogeneous mixing assumption shows differences in temperature, enthalpy, radiation losses, arc efficiency, and velocity at 400 A. Comparison with available experiments exhibits very good qualitative and quantitative agreement for the radial temperature and velocity profiles 2 mm downstream of the exit nozzle.

Slot-Antenna/Permanent-Magnet Device for Generating Plasma

NASA Technical Reports Server (NTRS)

Foster, John E.

2007-01-01

A device that includes a rectangular-waveguide/slot-antenna structure and permanent magnets has been devised as a means of generating a substantially uniform plasma over a relatively large area, using relatively low input power and a low gas flow rate. The device utilizes electron cyclotron resonance (ECR) excited by microwave power to efficiently generate plasma in a manner that is completely electrodeless in the sense that, in principle, there is no electrical contact between the plasma and the antenna. Plasmas generated by devices like this one are suitable for use as sources of ions and/or electrons for diverse material-processing applications (e.g., etching or deposition) and for ion thrusters. The absence of plasma/electrode contact essentially prevents plasma-induced erosion of the antenna, thereby also helping to minimize contamination of the plasma and of objects exposed to the plasma. Consequently, the operational lifetime of the rectangular-waveguide/ slot-antenna structure is long and the lifetime of the plasma source is limited by the lifetime of the associated charged-particle-extraction grid (if used) or the lifetime of the microwave power source. The device includes a series of matched radiating slot pairs that are distributed along the length of a plasma-source discharge chamber (see figure). This arrangement enables the production of plasma in a distributed fashion, thereby giving rise to a uniform plasma profile. A uniform plasma profile is necessary for uniformity in any electron- or ion-extraction electrostatic optics. The slotted configuration of the waveguide/ antenna structure makes the device scalable to larger areas and higher powers. All that is needed for scaling up is the attachment of additional matched radiating slots along the length of the discharge chamber. If it is desired to make the power per slot remain constant in scaling up, then the input microwave power must be increased accordingly. Unlike in prior ECR microwave plasma-generating devices, there is no need for an insulating window on the antenna. Such windows are sources of contamination and gradually become ineffective as they become coated with erosion products over time. These characteristics relegate prior ECR microwave plasma-generating devices to non-ion beam, non-deposition plasma applications. In contrast, the lack of need for an insulating window in the present device makes it possible to use the device in both ion-beam (including deposition) and electron-beam applications. The device is designed so that ECR takes place above each slot and the gradient of the magnetic field at each slot is enough to prevent backflow of plasma.

Hydrogen atom kinetics in capacitively coupled plasmas

NASA Astrophysics Data System (ADS)

Nunomura, Shota; Katayama, Hirotaka; Yoshida, Isao

2017-05-01

Hydrogen (H) atom kinetics has been investigated in capacitively coupled very high frequency (VHF) discharges at powers of 16-780 mW cm-2 and H2 gas pressures of 0.1-2 Torr. The H atom density has been measured using vacuum ultra violet absorption spectroscopy (VUVAS) with a micro-discharge hollow cathode lamp as a VUV light source. The measurements have been performed in two different electrode configurations of discharges: conventional parallel-plate diode and triode with an intermediate mesh electrode. We find that in the triode configuration, the H atom density is strongly reduced across the mesh electrode. The H atom density varies from ˜1012 cm-3 to ˜1010 cm-3 by crossing the mesh with 0.2 mm in thickness and 36% in aperture ratio. The fluid model simulations for VHF discharge plasmas have been performed to study the H atom generation, diffusion and recombination kinetics. The simulations suggest that H atoms are generated in the bulk plasma, by the electron impact dissociation (e + H2 \\to e + 2H) and the ion-molecule reaction (H2 + + H2 \\to {{{H}}}3+ + H). The diffusion of H atoms is strongly limited by a mesh electrode, and thus the mesh geometry influences the spatial distribution of the H atoms. The loss of H atoms is dominated by the surface recombination.

Highly ionized physical vapor deposition plasma source working at very low pressure

NASA Astrophysics Data System (ADS)

Stranak, V.; Herrendorf, A.-P.; Drache, S.; Cada, M.; Hubicka, Z.; Tichy, M.; Hippler, R.

2012-04-01

Highly ionized discharge for physical vapor deposition at very low pressure is presented in the paper. The discharge is generated by electron cyclotron wave resonance (ECWR) which assists with ignition of high power impulse magnetron sputtering (HiPIMS) discharge. The magnetron gun (with Ti target) was built into the single-turn coil RF electrode of the ECWR facility. ECWR assistance provides pre-ionization effect which allows significant reduction of pressure during HiPIMS operation down to p = 0.05 Pa; this is nearly more than an order of magnitude lower than at typical pressure ranges of HiPIMS discharges. We can confirm that nearly all sputtered particles are ionized (only Ti+ and Ti++ peaks are observed in the mass scan spectra). This corresponds well with high plasma density ne ˜ 1018 m-3, measured during the HiPIMS pulse.

On non-equilibrium atmospheric pressure plasma jets and plasma bullet

NASA Astrophysics Data System (ADS)

Lu, Xinpei

2012-10-01

Because of the enhanced plasma chemistry, atmospheric pressure nonequilibrium plasmas (APNPs) have been widely studied for several emerging applications such as biomedical applications. For the biomedical applications, plasma jet devices, which generate plasma in open space (surrounding air) rather than in confined discharge gaps only, have lots of advantages over the traditional dielectric barrier discharge (DBD) devices. For example, it can be used for root canal disinfection, which can't be realized by the traditional plasma device. On the other hand, currently, the working gases of most of the plasma jet devices are noble gases or the mixtures of the noble gases with small amount of O2, or air. If ambient air is used as the working gas, several serious difficulties are encountered in the plasma generation process. Amongst these are high gas temperatures and disrupting instabilities. In this presentation, firstly, a brief review of the different cold plasma jets developed to date is presented. Secondly, several different plasma jet devices developed in our lab are reported. The effects of various parameters on the plasma jets are discussed. Finally, one of the most interesting phenomena of APNP-Js, the plasma bullet is discussed and its behavior is described. References: [1] X. Lu, M. Laroussi, V. Puech, Plasma Sources Sci. Technol. 21, 034005 (2012); [2] Y. Xian, X. Lu, S. Wu, P. Chu, and Y. Pan, Appl. Phys. Lett. 100, 123702 (2012); [3] X. Pei, X. Lu, J. Liu, D. Liu, Y. Yang, K. Ostrikov, P. Chu, and Y. Pan, J. Phys. D 45, 165205 (2012).

Perspective: The physics, diagnostics, and applications of atmospheric pressure low temperature plasma sources used in plasma medicine

NASA Astrophysics Data System (ADS)

Laroussi, M.; Lu, X.; Keidar, M.

2017-07-01

Low temperature plasmas have been used in various plasma processing applications for several decades. But it is only in the last thirty years or so that sources generating such plasmas at atmospheric pressure in reliable and stable ways have become more prevalent. First, in the late 1980s, the dielectric barrier discharge was used to generate relatively large volume diffuse plasmas at atmospheric pressure. Then, in the early 2000s, plasma jets that can launch cold plasma plumes in ambient air were developed. Extensive experimental and modeling work was carried out on both methods and much of the physics governing such sources was elucidated. Starting in the mid-1990s, low temperature plasma discharges have been used as sources of chemically reactive species that can be transported to interact with biological media, cells, and tissues and induce impactful biological effects. However, many of the biochemical pathways whereby plasma affects cells remain not well understood. This situation is changing rather quickly because the field, known today as "plasma medicine," has experienced exponential growth in the last few years thanks to a global research community that engaged in fundamental and applied research involving the use of cold plasma for the inactivation of bacteria, dental applications, wound healing, and the destruction of cancer cells/tumors. In this perspective, the authors first review the physics as well as the diagnostics of the principal plasma sources used in plasma medicine. Then, brief descriptions of their biomedical applications are presented. To conclude, the authors' personal assessment of the present status and future outlook of the field is given.

Shunting arc plasma source for pure carbon ion beam.

PubMed

Koguchi, H; Sakakita, H; Kiyama, S; Shimada, T; Sato, Y; Hirano, Y

2012-02-01

A plasma source is developed using a coaxial shunting arc plasma gun to extract a pure carbon ion beam. The pure carbon ion beam is a new type of deposition system for diamond and other carbon materials. Our plasma device generates pure carbon plasma from solid-state carbon material without using a hydrocarbon gas such as methane gas, and the plasma does not contain any hydrogen. The ion saturation current of the discharge measured by a double probe is about 0.2 mA∕mm(2) at the peak of the pulse.

Shunting arc plasma source for pure carbon ion beam

DOE Office of Scientific and Technical Information (OSTI.GOV)

Koguchi, H.; Sakakita, H.; Kiyama, S.

2012-02-15

A plasma source is developed using a coaxial shunting arc plasma gun to extract a pure carbon ion beam. The pure carbon ion beam is a new type of deposition system for diamond and other carbon materials. Our plasma device generates pure carbon plasma from solid-state carbon material without using a hydrocarbon gas such as methane gas, and the plasma does not contain any hydrogen. The ion saturation current of the discharge measured by a double probe is about 0.2 mA/mm{sup 2} at the peak of the pulse.

In-package inhibition of E.coli 0157:H7 on bulk romaine lettuce using cold plasma

USDA-ARS?s Scientific Manuscript database

Dielectric barrier discharge atmospheric cold plasma (DACP) treatment was evaluated for the inactivation of Escherichia coli O157:H7, surface morphology, color, carbon dioxide generation, and weight loss of bulk Romaine lettuce in a commercial plastic clamshell container. The lettuce samples were pa...

Direct-current cathodic vacuum arc system with magnetic-field mechanism for plasma stabilization.

PubMed

Zhang, H-S; Komvopoulos, K

2008-07-01

Filtered cathodic vacuum arc (FCVA) deposition is characterized by plasma beam directionality, plasma energy adjustment via substrate biasing, macroparticle filtering, and independent substrate temperature control. Between the two modes of FCVA deposition, namely, direct current (dc) and pulsed arc, the dc mode yields higher deposition rates than the pulsed mode. However, maintaining the dc arc discharge is challenging because of its inherent plasma instabilities. A system generating a special configuration of magnetic field that stabilizes the dc arc discharge during film deposition is presented. This magnetic field is also part of the out-of-plane magnetic filter used to focus the plasma beam and prevent macroparticle film contamination. The efficiency of the plasma-stabilizing magnetic-field mechanism is demonstrated by the deposition of amorphous carbon (a-C) films exhibiting significantly high hardness and tetrahedral carbon hybridization (sp3) contents higher than 70%. Such high-quality films cannot be produced by dc arc deposition without the plasma-stabilizing mechanism presented in this study.

Transient effects in beam-plasma interactions in a space simulation chamber stimulated by a fast pulse electron gun

NASA Technical Reports Server (NTRS)

Raitt, W. J.; Banks, P. M.; Denig, W. F.; Anderson, H. R.

1982-01-01

Interest in the interaction of electron beams with plasma generated by ionization caused by the primary electron beam was stimulated by the need to develop special vacuum tubes to operate in the kMHz frequency region. The experiments of Getty and Smullin (1963) indicated that the interaction of an energetic electron beam with its self-produced plasma resulted in the emission of wave energy over a wide range of frequencies associated with cyclotron and longitudinal plasma instabilities. This enhanced the thermal plasma density in the vicinity of the beam, and the term Beam-Plasma Discharge (BPD) was employed to described this phenomenon. The present investigation is concerned with some of the transient phenomena associated with wave emission during the beam switch-on and switch-off periods. Results are presented on the changes in electron energy spectra on a time scale of tens of milliseconds following beam switch-on. The results are discussed in terms of the beam plasma discharge phenomenon.

Characterization of an atmospheric pressure air plasma source for polymer surface modification

NASA Astrophysics Data System (ADS)

Yang, Shujun; Tang, Jiansheng

2013-10-01

An atmospheric pressure air plasma source was generated through dielectric barrier discharge (DBD). It was used to modify polyethyleneterephthalate (PET) surfaces with very high throughput. An equivalent circuit model was used to calculate the peak average electron density. The emission spectrum from the plasma was taken and the main peaks in the spectrum were identified. The ozone density in the down plasma region was estimated by Absorption Spectroscopy. NSF and ARC-ODU

A Plasma Focus Device with a 2-MA Discharge Current as a Hard X-Ray Source

NASA Astrophysics Data System (ADS)

Yurkov, D. I.; Dulatov, A. K.; Lemeshko, B. D.; Andreev, D. A.; Golikov, A. V.; Mikhailov, Yu. V.; Prokuratov, I. A.; Selifanov, A. N.; Fatiev, T. S.

2018-04-01

A device based on a pulsed current generator with capacitive energy storage loaded on a plasma focus (PF) chamber is described. The device provides a discharge current amplitude of up to 2 MA in the PF chamber at a stored energy in the capacitor bank of up to 150 kJ. The PF chamber is designed to study hard X-ray (HXR) emission. It has windows for output of HXR emission in the cathode direction, as well as a special insert for output of HXR emission into the anode cavity. A study of operation of the chamber as a part of the setup with the use of various X-ray targets on the anode has been carried out. At a discharge current of 1.5MA, an HXR pulse with an average duration of 16 ns and energy spectrum from 10 to 200 keV, which provides an absorbed dose in the irradiated samples on the order of 1 Sv, is generated in the PF chamber.

Aqueous reactive species induced by a PCB surface micro-discharge air plasma device: a quantitative study

NASA Astrophysics Data System (ADS)

Chen, Chen; Li, Fanying; Chen, Hai-Lan; Kong, Michael G.

2017-11-01

This paper presents a quantitative investigation on aqueous reactive species induced by air plasma generated from a printed circuit board surface micro-discharge (SMD) device. Under the conditions amenable for proliferation of mammalian cells, concentrations of ten types of reactive oxygen and nitrogen species (RONS) in phosphate buffering solution (PBS) are measured by chemical fluorescent assays and electron spin resonance spectroscopy (ESR). Results show that concentrations of several detected RNS (NO2- , NO3- , peroxynitrites, and NO2\\centerdot ) are higher than those of ROS (H2O2, O2\\centerdot - , and 1O2) in the air plasma treated solution. Concentrations of NO3- can reach 150 times of H2O2 with 60 s plasma treatment. For short-lived species, the air plasma generates more copious peroxynitrite than other RONS including NO2\\centerdot , O2\\centerdot - , 1O2, and N{{O}\\centerdot } in PBS. In addition, the existence of reaction between H2O2 and NO2- /HNO2 to produce peroxynitrite is verified by the chemical scavenger experiments. The reaction relations between detected RONS are also discussed.

Influence of electron injection into 27 cm audio plasma cell on the plasma diagnostics

DOE Office of Scientific and Technical Information (OSTI.GOV)

Haleem, N. A.; Ragheb, M. S.; Zakhary, S. G.

2013-08-15

In this article, the plasma is created in a Pyrex tube (L = 27 cm, φ= 4 cm) as a single cell, by a capacitive audio frequency (AF) discharge (f = 10–100 kHz), at a definite pressure of ∼0.2 Torr. A couple of tube linear and deviating arrangements show plasma characteristic conformity. The applied AF plasma and the injection of electrons into two gas mediums Ar and N{sub 2} revealed the increase of electron density at distinct tube regions by one order to attain 10{sup 13}/cm{sup 3}. The electrons temperature and density strengths are in contrast to each other. Whilemore » their distributions differ along the plasma tube length, they show a decaying sinusoidal shape where their peaks position varies by the gas type. The electrons injection moderates electron temperature and expands their density. The later highest peak holds for the N{sub 2} gas, at electrons injection it changes to hold for the Ar. The sinusoidal decaying density behavior generates electric fields depending on the gas used and independent of tube geometry. The effect of the injected electrons performs a responsive impact on electrons density not attributed to the gas discharge. Analytical tools investigate the interaction of the plasma, the discharge current, and the gas used on the electrodes. It points to the emigration of atoms from each one but for greater majority they behave to a preferred direction. Meanwhile, only in the linear regime, small percentage of atoms still moves in reverse direction. Traces of gas atoms revealed on both electrodes due to sheath regions denote lack of their participation in the discharge current. In addition, atoms travel from one electrode to the other by overcoming the sheaths regions occurring transportation of particles agglomeration from one electrode to the other. The electrons injection has contributed to increase the plasma electron density peaks. These electrons populations have raised the generated electrostatic fields assisting the elemental ions emigration to a preferred electrode direction. Regardless of plasma electrodes positions and plasma shape, ions can be departed from one electrode to deposit on the other one. In consequence, as an application the AF plasma type can enhance the metal deposition from one electrode to the other.« less

Autonomous Method and System for Minimizing the Magnitude of Plasma Discharge Current Oscillations in a Hall Effect Plasma Device

NASA Technical Reports Server (NTRS)

Hruby, Vladimir (Inventor); Demmons, Nathaniel (Inventor); Ehrbar, Eric (Inventor); Pote, Bruce (Inventor); Rosenblad, Nathan (Inventor)

2014-01-01

An autonomous method for minimizing the magnitude of plasma discharge current oscillations in a Hall effect plasma device includes iteratively measuring plasma discharge current oscillations of the plasma device and iteratively adjusting the magnet current delivered to the plasma device in response to measured plasma discharge current oscillations to reduce the magnitude of the plasma discharge current oscillations.

Transmission characteristics of microwave in a glow-discharge dusty plasma

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jia, Jieshu; Yuan, Chengxun, E-mail: yuancx@hit.edu.cn; Gao, Ruilin

2016-07-15

In this study, the propagation characteristics of electromagnetic wave in a glow discharge plasma with dust particles are experimentally investigated. A helium alternating current glow discharge plasmas have been successfully generated. Measurements of the plasma parameters using Langmuir probes, in the absence of dust particles, provide plasma densities (n{sub e}) of 10{sup 17 }m{sup −3} and electron temperatures (T{sub e}) ranging from 2 to 4 eV. Dusty plasmas are made by adding 30 nm radius aluminum oxide (Al{sub 2}O{sub 3}) particles into the helium plasma. The density of the dust particle (n{sub d}) in the device is about 10{sup 11}–10{sup 12 }m{sup −3}. Themore » propagation characteristics of electromagnetic waves are determined by a vector network analyzer with 4–6 GHz antennas. An apparent attenuation by the dust is observed, and the measured attenuation data are approximately in accordance with the theoretical calculations. The effects of gas pressure and input power on the propagation are also investigated. Results show that the transmission attenuation increases with the gas pressure and input power, the charged dust particles play a significant role in the microwave attenuation.« less

Dielectric barrier discharge plasma actuator for flow control

NASA Astrophysics Data System (ADS)

Opaits, Dmitry Florievich

Electrohydrodynamic (EHD) and magnetohydrodynamic phenomena are being widely studied for aerodynamic applications. The major effects of these phenomena are heating of the gas, body force generation, and enthalpy addition or extraction, [1, 2, 3]. In particular, asymmetric dielectric barrier discharge (DBD) plasma actuators are known to be effective EHD device in aerodynamic control, [4, 5]. Experiments have demonstrated their effectiveness in separation control, acoustic noise reduction, and other aeronautic applications. In contrast to conventional DBD actuators driven by sinusoidal voltages, we proposed and used a voltage profile consisting of nanosecond pulses superimposed on dc bias voltage. This produces what is essentially a non-self-sustained discharge: the plasma is generated by repetitive short pulses, and the pushing of the gas occurs primarily due to the bias voltage. The advantage of this non-self-sustained discharge is that the parameters of ionizing pulses and the driving bias voltage can be varied independently, which adds flexibility to control and optimization of the actuators performance. Experimental studies were conducted of a flow induced in a quiescent room air by a single DBD actuator. A new approach for non-intrusive diagnostics of plasma actuator induced flows in quiescent gas was proposed, consisting of three elements coupled together: the Schlieren technique, burst mode of plasma actuator operation, and 2-D numerical fluid modeling. During the experiments, it was found that DBD performance is severely limited by surface charge accumulation on the dielectric. Several ways to mitigate the surface charge were found: using a reversing DC bias potential, three-electrode configuration, slightly conductive dielectrics, and semi conductive coatings. Force balance measurements proved the effectiveness of the suggested configurations and advantages of the new voltage profile (pulses+bias) over the traditional sinusoidal one at relatively low voltages. In view of practical applications certain questions have been also addressed, such as electrodynamic effects which accompany scaling of the actuators to real size models, and environmental effects of ozone production by the plasma actuators.

Method and apparatus for detecting halogenated hydrocarbons

DOEpatents

Monagle, Matthew; Coogan, John J.

1997-01-01

A halogenated hydrocarbon (HHC) detector is formed from a silent discharge (also called a dielectric barrier discharge) plasma generator. A silent discharge plasma device receives a gas sample that may contain one or more HHCs and produces free radicals and excited electrons for oxidizing the HHCs in the gas sample to produce water, carbon dioxide, and an acid including halogens in the HHCs. A detector is used to sensitively detect the presence of the acid. A conductivity cell detector combines the oxidation products with a solvent where dissociation of the acid increases the conductivity of the solvent. The conductivity cell output signal is then functionally related to the presence of HHCs in the gas sample. Other detectors include electrochemical cells, infrared spectrometers, and negative ion mobility spectrometers.

Modeling of non-thermal plasma in flammable gas mixtures

NASA Astrophysics Data System (ADS)

Napartovich, A. P.; Kochetov, I. V.; Leonov, S. B.

2008-07-01

An idea of using plasma-assisted methods of fuel ignition is based on non-equilibrium generation of chemically active species that speed up the combustion process. It is believed that gain in energy consumed for combustion acceleration by plasmas is due to the non-equilibrium nature of discharge plasma, which allows radicals to be produced in an above-equilibrium amount. Evidently, the size of the effect is strongly dependent on the initial temperature, pressure, and composition of the mixture. Of particular interest is comparison between thermal ignition of a fuel-air mixture and non-thermal plasma initiation of the combustion. Mechanisms of thermal ignition in various fuel-air mixtures have been studied for years, and a number of different mechanisms are known providing an agreement with experiments at various conditions. The problem is -- how to conform thermal chemistry approach to essentially non-equilibrium plasma description. The electric discharge produces much above-equilibrium amounts of chemically active species: atoms, radicals and ions. The point is that despite excess concentrations of a number of species, total concentration of these species is far below concentrations of the initial gas mixture. Therefore, rate coefficients for reactions of these discharge produced species with other gas mixture components are well known quantities controlled by the translational temperature, which can be calculated from the energy balance equation taking into account numerous processes initiated by plasma. A numerical model was developed combining traditional approach of thermal combustion chemistry with advanced description of the plasma kinetics based on solution of electron Boltzmann equation. This approach allows us to describe self-consistently strongly non-equilibrium electric discharge in chemically unstable (ignited) gas. Equations of pseudo-one-dimensional gas dynamics were solved in parallel with a system of thermal chemistry equations, kinetic equations for charged particles (electrons, positive and negative ions), and with the electric circuit equation. The electric circuit comprises power supply, ballast resistor connected in series with the discharge and capacity. Rate coefficients for electron-assisted reactions were calculated from solving the two-term spherical harmonic expansion of the Boltzmann equation. Such an approach allows us to describe influence of thermal chemistry reactions (burning) on the discharge characteristics. Results of comparison between the discharge and thermal ignition effects for mixtures of hydrogen or ethylene with dry air will be reported. Effects of acceleration of ignition by discharge plasma will be analyzed. In particular, the role of singlet oxygen produced effectively in the discharge in ignition speeding up will be discussed.

Effects of E × B drift on electron transport across the magnetic field in a miniature microwave discharge neutralizer

NASA Astrophysics Data System (ADS)

Hiramoto, Kenta; Nakagawa, Yuichi; Koizumi, Hiroyuki; Takao, Yoshinori

2017-06-01

Using a three-dimensional particle-in-cell model, electron transport across a magnetic field has been investigated by obtaining the time-varying electric field and plasma parameters in a miniature microwave discharge neutralizer. The size of the neutralizer is 20 × 20 × 4 mm3. Ring-shaped antenna producing 4.2 GHz microwaves and permanent magnets for xenon plasma discharges are present inside. There are four orifices for electron extraction. The simulation area consists of both the discharge chamber and the vacuum region for the extraction. The numerical results show that radial striped patterns occur where the peak electron density is obtained, and the patterns seem to rotate in the azimuthal direction. This characteristic structure is very similar to recent results obtained in Hall thrusters and is probably due to the electron drift instability. Owing to the plasma structure, the azimuthal electric field is generated, which results in the E × B drift velocity in the axial direction with the radial magnetic field of the permanent magnets. This E × B drift velocity is a key factor in the electron transport across the magnetic field, leading to the electron extraction from the discharge chamber.

A note on supersonic flow control with nanosecond plasma actuator

NASA Astrophysics Data System (ADS)

Zheng, J. G.; Cui, Y. D.; Li, J.; Khoo, B. C.

2018-04-01

A concept study on supersonic flow control using nanosecond pulsed plasma actuator is conducted by means of numerical simulation. The nanosecond plasma discharge is characterized by the generation of a micro-shock wave in ambient air and a residual heat in the discharge volume arising from the rapid heating of near-surface gas by the quick discharge. The residual heat has been found to be essential for the flow separation control over aerodynamic bodies like airfoil and backward-facing step. In this study, novel experiment is designed to utilize the other flow feature from discharge, i.e., instant shock wave, to control supersonic flow through shock-shock interaction. Both bow shock in front of a blunt body and attached shock anchored at the tip of supersonic projectile are manipulated via the discharged-induced shock wave in an appropriate manner. It is observed that drag on the blunt body is reduced appreciably. Meanwhile, a lateral force on sharp-edged projectile is produced, which can steer the body and give it an effective angle of attack. This opens a promising possibility for extending the applicability of this flow control technique in supersonic flow regime.

Experimental study of low-temperature plasma of electrical discharges with liquid electrodes

NASA Astrophysics Data System (ADS)

Zheltukhin, Viktor; Gaisin, Almaz

2016-09-01

Results of the experimental research of discharge between the liquid jet cathode (LJC) and the metal anode are presented. The discharge was studied over the voltage range U = 100 - 600 V, discharge current range I = 0 . 1 - 0 . 25 A, external pressure range P =105 Pa, discharge power Pd = 10 - 150 W. We used the techniques of infrared thermography and spectral measurements. Schlieren's photography is applied for describing the processes in liquid and gas phase. Results of the experimental researches of discharge current-voltage characteristic (CVC), the surface temperature distribution both on the LJC and the metal anode, a spectral measurements are showed. Effects of action both of breakdown and discharge on the jet flow as well as on the air flow near the discharge are described. It is found that the discharge CVC has an ascending behavior due to increase of plasma current density. The discharge is generated on the borders between the LJC and the metal anode as well as along the LJC misshaping this one. It is established that both the convection streams and an electrolyte drops are formed during the discharge burn. It is found that the discharge temperature in the vicinity of electrode surface reaches T 348 K. The work was funded by RFBR, according to the research projects No.,14-01-0755.

Susceptibility of Staphylococcus aureus biofilms to reactive discharge gases.

PubMed

Traba, Christian; Liang, Jun F

2011-08-01

Formation of bacterial biofilms at solid-liquid interfaces creates numerous problems in both industrial and biomedical sciences. In this study, the susceptibility of Staphylococcus aureus biofilms to discharge gas generated from plasma was tested. It was found that despite distinct chemical/physical properties, discharge gases from oxygen, nitrogen, and argon demonstrated very potent and almost the same anti-biofilm activity. The bacterial cells in S. aureus biofilms were killed (>99.9%) by discharge gas within minutes of exposure. Under optimal experimental conditions, no bacteria and biofilm re-growth from discharge gas treated biofilms was found. Further studies revealed that the anti-biofilm activity of the discharge gas occurred by two distinct mechanisms: (1) killing bacteria in biofilms by causing severe cell membrane damage, and (2) damaging the extracellular polymeric matrix in the architecture of the biofilm to release biofilm from the surface of the solid substratum. Information gathered from this study provides an insight into the anti-biofilm mechanisms of plasma and confirms the applications of discharge gas in the treatment of biofilms and biofilm related bacterial infections.

Pulsed high voltage electric discharge disinfection of microbially contaminated liquids.

PubMed

Anpilov, A M; Barkhudarov, E M; Christofi, N; Kop'ev, V A; Kossyi, I A; Taktakishvili, M I; Zadiraka, Y

2002-01-01

To examine the use of a novel multielectrode slipping surface discharge (SSD) treatment system, capable of pulsed plasma discharge directly in water, in killing micro-organisms. Potable water containing Escherichia coli and somatic coliphages was treated with pulsed electric discharges generated by the SSD. The SSD system was highly efficient in the microbial disinfection of water with a low energy utilization (eta approximately 10-4 kW h l-1). The SSD treatment was effective in the destruction of E. coli and its coliphages through the generation of u.v. radiation, ozone and free radicals. The non-thermal treatment method can be used for the eradication of micro-organisms in a range of contaminated liquids, including milk, negating the use of pasteurization. The method utilizes multipoint electric discharges capable of treating large volumes of liquid under static and flowing regimes.

Cytotoxicity of cancer HeLa cells sensitivity to normal MCF10A cells in cultivations with cell culture medium treated by microwave-excited atmospheric pressure plasmas

NASA Astrophysics Data System (ADS)

Takahashi, Yohei; Taki, Yusuke; Takeda, Keigo; Hashizume, Hiroshi; Tanaka, Hiromasa; Ishikawa, Kenji; Hori, Masaru

2018-03-01

Cytotoxic effects of human epithelial carcinoma HeLa cells sensitivity to human mammary epithelial MCF10A cells appeared in incubation with the plasma-activated medium (PAM), where the cell culture media were irradiated with the hollow-shaped contact of a continuously discharged plasma that was sustained by application of a microwave power under Ar gas flow at atmospheric pressure. The discharged plasma had an electron density of 7  ×  1014 cm-3. As the nozzle exit to the plasma source was a distance of 5 mm to the medium, concentrations of 180 µM for H2O2 and 77 µM for NO2- were generated in the PAM for 30 s irradiation, resulting in the control of irradiation periods for aqueous H2O2 with a generation rate of 6.0 µM s-1, and nitrite ion (NO2- ) with a rate of 2.2 µM s-1. Effective concentrations of H2O2 and NO2- for the antitumor effects were revealed in the microwave-excited PAM, with consideration of the complicated reactions at the plasma-liquid interfaces.

Plasma application for detoxification of Jatropha phorbol esters

NASA Astrophysics Data System (ADS)

Kongmany, S.; Matsuura, H.; Furuta, M.; Okuda, S.; Imamura, K.; Maeda, Y.

2013-06-01

Atmospheric pressure non-thermal dielectric barrier discharge (DBD) plasma generated by helium gas at high voltage and input power of about 50 W was first applied to detoxification of Jatropha curcas phorbol esters (J. PEs) as well as standard phorbol ester (4β-12-O-tetradecanoyl phorbol-13-acetate, TPA) in water and methanol. Plasma irradiation on the solution sample was conducted for 15 min. In aqueous solution, only 16% of TPA was degraded and complete degradation of J. PEs was observed. On the contrary, complete degradation of both TPA and J. PEs in methanol was achieved by the same plasma irradiation condition. Hydroxyl radical (•OH) generated by plasma irradiation of the solution is expected as the main radical inducing the degradation of PEs.

Synthesis and characteristics of Ag/Pt bimetallic nanocomposites by arc-discharge solution plasma processing.

PubMed

Pootawang, Panuphong; Saito, Nagahiro; Takai, Osamu; Lee, Sang-Yul

2012-10-05

Arc discharge in solution, generated by applying a high voltage of unipolar pulsed dc to electrodes of Ag and Pt, was used as a method to form Ag/Pt bimetallic nanocomposites via electrode erosion by the effects of the electric arc at the cathode (Ag rod) and the sputtering at the anode (Pt rod). Ag/Pt bimetallic nanocomposites were formed as colloidal particles dispersed in solution via the reduction of hydrogen radicals generated during discharge without the addition of chemical precursor or reducing agent. At a discharge time of 30 s, the fine bimetallic nanoparticles with a mean particle size of approximately 5 nm were observed by transmission electron microscopy (TEM). With increasing discharge time, the bimetallic nanoparticle size tended to increase by forming an agglomeration. The presence of the relatively small amount of Pt dispersed in the Ag matrix could be observed by the analytical mapping mode of energy-dispersive x-ray spectroscopy and high-resolution TEM. This demonstrated that the synthesized particle was in the form of a nanocomposite. No contamination of other chemical substances was detected by x-ray photoelectron spectroscopy. Hence, solution plasma could be a clean and simple process to effectively synthesize Ag/Pt bimetallic nanocomposites and it is expected to be widely applicable in the preparation of several types of nanoparticle.

Dynamic generation of supercritical water fluid in a strong electrical discharge in a liquid

NASA Astrophysics Data System (ADS)

Antonov, V.; Kalinin, N.; Kovalenko, A.

2016-11-01

A new impetus for the development of electro physics is associated with using different types of electrical discharges in biology and medicine. These applications are based on their energetic and non-toxic factors affecting the medium on a cellular level. For the study of such processes, a mathematical model of a high-current low-temperature Z-discharge in a liquid, forming by the electrical explosion of a thin-walled metal shell, connected to a pulsed high-voltage generator, has been developed. High efficiency energy conversion, introduced into the plasma discharge to the energy of fluid motion, provides various bio chemical applications of such physical processes. The investigation is conducted through numerical solution of one-dimensional single-temperature non-stationary equations of radiation magneto hydrodynamics, one way describing the evolution of hydrodynamic, thermal and electrical characteristics of the medium throughout the area under consideration. The electrical approximation based on the assumption that the electric field in the discharge has a uniform distribution. The results are presented as a function of the electric current and the plasma channel length of time, as well as the temperature and pressure distributions at different time points along the radius of the cylindrical region in which the explosion occurs.

Impurities, temperature, and density in a miniature electrostatic plasma and current source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Den Hartog, D.J.; Craig, D.J.; Fiksel, G.

1996-10-01

We have spectroscopically investigated the Sterling Scientific miniature electrostatic plasma source-a plasma gun. This gun is a clean source of high density (10{sup 19} - 10{sup 20} m{sup -3}), low temperature (5 - 15 eV) plasma. A key result of our investigation is that molybdenum from the gun electrodes is largely trapped in the internal gun discharge; only a small amount escapes in the plasma flowing out of the gun. In addition, the gun plasma parameters actually improve (even lower impurity contamination and higher ion temperature) when up to 1 kA of electron current is extracted from the gun viamore » the application of an external bias. This improvement occurs because the internal gun anode no longer acts as the current return for the internal gun discharge. The gun plasma is a virtual plasma electrode capable of sourcing an electron emission current density of 1 kA/cm{sup 2}. The high emission current, small size (3 - 4 cm diameter), and low impurity generation make this gun attractive for a variety of fusion and plasma technology applications.« less

Innovative approach for benzene degradation using hybrid surface/packed-bed discharge plasmas.

PubMed

Jiang, Nan; Lu, Na; Shang, Kefeng; Li, Jie; Wu, Yan

2013-09-03

An innovative plasma reactor, which generates hybrid surface/packed-bed discharge (HSPBD) plasmas, was employed for the degradation of benzene. The HSPBD reactor was found to display remarkably better benzene degradation, mineralization, and energy performance than surface or packed-bed discharge reactors alone. The degradation efficiency, CO2 selectivity, and energy yield in the HSPBD reactor were 21%, 11%, and 3.9 g kWh-1 higher, respectively, than in a surface discharge reactor and 30%, 21%, and 5.5 g kWh-1 higher, respectively, than in a packed-bed discharge reactor operated at 280 J L-1. Particularly, the benzene degradation in the HSPBD reactor exhibited an unambiguous synergistic enhancement rather than a simple additive effect using the surface discharge and packed-bed discharge reactors. Moreover, in the HSPBD reactor, the formation of byproducts, such as NO2, was suppressed, while O3 was promoted. The use of N2 as the carrier gas was found to be effective for benzene degradation because of the fast reaction rate of N2(A3∑u+) with benzene, and oxygen species derived from the dissociation of O2 were found to be significant in the mineralization process. Thus, the addition of O2 to N2 allows for efficient degradation of benzene, and the optimized amount of O2 was determined to be 3%.

Quantification of the effect of surface heating on shock wave modification by a plasma actuator in a low-density supersonic flow over a flat plate

NASA Astrophysics Data System (ADS)

Joussot, Romain; Lago, Viviana; Parisse, Jean-Denis

2015-05-01

This paper describes experimental and numerical investigations focused on the shock wave modification induced by a dc glow discharge. The model is a flat plate in a Mach 2 air flow, equipped with a plasma actuator composed of two electrodes. A weakly ionized plasma was created above the plate by generating a glow discharge with a negative dc potential applied to the upstream electrode. The natural flow exhibited a shock wave with a hyperbolic shape. Pitot measurements and ICCD images of the modified flow revealed that when the discharge was ignited, the shock wave angle increased with the discharge current. The spatial distribution of the surface temperature was measured with an IR camera. The surface temperature increased with the current and decreased along the model. The temperature distribution was reproduced experimentally by placing a heating element instead of the active electrode, and numerically by modifying the boundary condition at the model surface. For the same surface temperature, experimental investigations showed that the shock wave angle was lower with the heating element than for the case with the discharge switched on. The results show that surface heating is responsible for roughly 50 % of the shock wave angle increase, meaning that purely plasma effects must also be considered to fully explain the flow modifications observed.

Transition in discharge plasma of Hall thruster type in presence of secondary electron emissive surface

NASA Astrophysics Data System (ADS)

Schweigert, I. V.; Yadrenkin, M. A.; Fomichev, V. P.

2017-11-01

Modification of the sheath structure near the emissive plate placed in magnetized DC discharge plasma of Hall thruster type was studied in the experiment and in kinetic simulations. The plate is made from Al2O3 which has enhanced secondary electron emission yield. The energetic electrons emitted by heated cathode provide the volume ionization and the secondary electron emission from the plate. An increase of the electron beam energy leads to an increase of the secondary electron generation, which initiates the transition in sheath structure over the emissive plate.

Application of a Bonner sphere spectrometer for determination of the energy spectra of neutrons generated by ≈1 MJ plasma focus.

PubMed

Králík, M; Krása, J; Velyhan, A; Scholz, M; Ivanova-Stanik, I M; Bienkowska, B; Miklaszewski, R; Schmidt, H; Řezáč, K; Klír, D; Kravárik, J; Kubeš, P

2010-11-01

The spectra of neutrons outside the plasma focus device PF-1000 with an upper energy limit of ≈1 MJ was measured using a Bonner spheres spectrometer in which the active detector of thermal neutrons was replaced by nine thermoluminescent chips. As an a priori spectrum for the unfolding procedure, the spectrum calculated by means of the Monte Carlo method with a simplified model of the discharge chamber was selected. Differences between unfolded and calculated spectra are discussed with respect to properties of the discharge vessel and the laboratory layout.

Integration and Test Flight Validation Plans for the Pulsed Plasma Thruster Experiment on EO- 1

NASA Technical Reports Server (NTRS)

Zakrzwski, Charles; Benson, Scott; Sanneman, Paul; Hoskins, Andy; Bauer, Frank H. (Technical Monitor)

2002-01-01

The Pulsed Plasma Thruster (PPT) Experiment on the Earth Observing One (EO-1) spacecraft has been designed to demonstrate the capability of a new generation PPT to perform spacecraft attitude control. The PPT is a small, self-contained pulsed electromagnetic propulsion system capable of delivering high specific impulse (900-1200 s), very small impulse bits (10-1000 uN-s) at low average power (less than 1 to 100 W). Teflon fuel is ablated and slightly ionized by means of a capacitative discharge. The discharge also generates electromagnetic fields that accelerate the plasma by means of the Lorentz Force. EO-1 has a single PPT that can produce thrust in either the positive or negative pitch direction. The flight validation has been designed to demonstrate of the ability of the PPT to provide precision pointing accuracy, response and stability, and confirmation of benign plume and EMI effects. This paper will document the success of the flight validation.

High Frequency Plasma Generators for Ion Thrusters

NASA Technical Reports Server (NTRS)

Divergilio, W. F.; Goede, H.; Fosnight, V. V.

1981-01-01

The results of a one year program to experimentally adapt two new types of high frequency plasma generators to Argon ion thrusters and to analytically study a third high frequency source concept are presented. Conventional 30 cm two grid ion extraction was utilized or proposed for all three sources. The two plasma generating methods selected for experimental study were a radio frequency induction (RFI) source, operating at about 1 MHz, and an electron cyclotron heated (ECH) plasma source operating at about 5 GHz. Both sources utilize multi-linecusp permanent magnet configurations for plasma confinement. The plasma characteristics, plasma loading of the rf antenna, and the rf frequency dependence of source efficiency and antenna circuit efficiency are described for the RFI Multi-cusp source. In a series of tests of this source at Lewis Research Center, minimum discharge losses of 220+/-10 eV/ion were obtained with propellant utilization of .45 at a beam current of 3 amperes. Possible improvement modifications are discussed.

Mach 5 bow shock control by a nanosecond pulse surface dielectric barrier discharge

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nishihara, M.; Takashima, K.; Rich, J. W.

2011-06-15

Bow shock perturbations in a Mach 5 air flow, produced by low-temperature, nanosecond pulse, and surface dielectric barrier discharge (DBD), are detected by phase-locked schlieren imaging. A diffuse nanosecond pulse discharge is generated in a DBD plasma actuator on a surface of a cylinder model placed in air flow in a small scale blow-down supersonic wind tunnel. Discharge energy coupled to the actuator is 7.3-7.8 mJ/pulse. Plasma temperature inferred from nitrogen emission spectra is a few tens of degrees higher than flow stagnation temperature, T = 340 {+-} 30 K. Phase-locked Schlieren images are used to detect compression waves generatedmore » by individual nanosecond discharge pulses near the actuator surface. The compression wave propagates upstream toward the baseline bow shock standing in front of the cylinder model. Interaction of the compression wave and the bow shock causes its displacement in the upstream direction, increasing shock stand-off distance by up to 25%. The compression wave speed behind the bow shock and the perturbed bow shock velocity are inferred from the Schlieren images. The effect of compression waves generated by nanosecond discharge pulses on shock stand-off distance is demonstrated in a single-pulse regime (at pulse repetition rates of a few hundred Hz) and in a quasi-continuous mode (using a two-pulse sequence at a pulse repetition rate of 100 kHz). The results demonstrate feasibility of hypersonic flow control by low-temperature, repetitive nanosecond pulse discharges.« less

Plasma-filled diode based on the coaxial gun

NASA Astrophysics Data System (ADS)

Zherlitsyn, A. A.; Kovalchuk, B. M.; Pedin, N. N.

2012-10-01

The paper presents the results of studies of a coaxial gun for a plasma-filled electron diode. Effects of the discharge channel diameter and gun current on characteristics of the plasma and pulse generated in the diode were investigated. The electron beam with maximum energy of ≥1 MeV at the current of ≈100 kA was obtained in the experiments with a plasma-filled diode. The energy of ≈5 kJ with the peak power of ≥100 GW dissipated in the diode.

Plasma-filled diode based on the coaxial gun.

PubMed

Zherlitsyn, A A; Kovalchuk, B M; Pedin, N N

2012-10-01

The paper presents the results of studies of a coaxial gun for a plasma-filled electron diode. Effects of the discharge channel diameter and gun current on characteristics of the plasma and pulse generated in the diode were investigated. The electron beam with maximum energy of ≥1 MeV at the current of ≈100 kA was obtained in the experiments with a plasma-filled diode. The energy of ≈5 kJ with the peak power of ≥100 GW dissipated in the diode.

Inactivation of Escherichia coli and Staphylococcus aureus on contaminated perilla leaves by Dielectric Barrier Discharge (DBD) plasma treatment.

PubMed

Ji, Sang Hye; Ki, Se Hoon; Ahn, Ji Ho; Shin, Jae Ho; Hong, Eun Jeong; Kim, Yun Ji; Choi, Eun Ha

2018-04-02

This study focused on sterilization methods for the reduction of microorganisms on perilla leaves by cylinder type Dielectric Barrier Discharge (DBD) plasma with underwater bubbler treatment. S. aureus and E. coli in a suspension were reduced to less than 3.4 and 0.5 log CFU/ml after the plasma treatment for 3 min, respectively. On the perilla leaves, they were also reduced to 4.8 and 1.6 log CFU/ml after the plasma treatment, respectively. The S. aureus and E. coli bacterial cell wall was damaged by the plasma treatment evident by scanning electron microscopic analysis. The observed infrared bands of the FTIR spectra demonstrated changes in protein, lipid, polysaccharide, polyphosphate group and other carbohydrate functionalities of plasma treated bacteria and untreated bacterial cell membranes. The degradation of the constituent bonds of the bacterial cell membrane by RONS generated from plasma destroys the DNA, RNA, and proteins within the cell, and may eventually cause cell death. In this study, H 2 O 2 (13.68 μM) and NO 3 (138 μM), which are the main factors generated by plasma, proved to have a bactericidal effect by inducing lipid peroxidation of bacterial cell membranes. In conclusion, cylinder type DBD plasma with underwater bubbler can be used as an environmentally friendly food disinfection device in cleaning processes of the food industry. Copyright © 2018 Elsevier Inc. All rights reserved.

Atmospheric-pressure plasma jets: Effect of gas flow, active species, and snake-like bullet propagation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wu, S.; Wang, Z.; Huang, Q.

2013-02-15

Cold atmospheric-pressure plasma jets have recently attracted enormous interest owing to numerous applications in plasma biology, health care, medicine, and nanotechnology. A dedicated study of the interaction between the upstream and downstream plasma plumes revealed that the active species (electrons, ions, excited OH, metastable Ar, and nitrogen-related species) generated by the upstream plasma plume enhance the propagation of the downstream plasma plume. At gas flows exceeding 2 l/min, the downstream plasma plume is longer than the upstream plasma plume. Detailed plasma diagnostics and discharge species analysis suggest that this effect is due to the electrons and ions that are generatedmore » by the upstream plasma and flow into the downstream plume. This in turn leads to the relatively higher electron density in the downstream plasma. Moreover, high-speed photography reveals a highly unusual behavior of the plasma bullets, which propagate in snake-like motions, very differently from the previous reports. This behavior is related to the hydrodynamic instability of the gas flow, which results in non-uniform distributions of long-lifetime active species in the discharge tube and of surface charges on the inner surface of the tube.« less

Air plasma treatment of liquid covered tissue: long timescale chemistry

NASA Astrophysics Data System (ADS)

Lietz, Amanda M.; Kushner, Mark J.

2016-10-01

Atmospheric pressure plasmas have shown great promise for the treatment of wounds and cancerous tumors. In these applications, the sample is usually covered by a thin layer of a biological liquid. The reactive oxygen and nitrogen species (RONS) generated by the plasma activate and are processed by the liquid before the plasma produced activation reaches the tissue. The synergy between the plasma and the liquid, including evaporation and the solvation of ions and neutrals, is critical to understanding the outcome of plasma treatment. The atmospheric pressure plasma sources used in these procedures are typically repetitively pulsed. The processes activated by the plasma sources have multiple timescales—from a few ns during the discharge pulse to many minutes for reactions in the liquid. In this paper we discuss results from a computational investigation of plasma-liquid interactions and liquid phase chemistry using a global model with the goal of addressing this large dynamic range in timescales. In modeling air plasmas produced by a dielectric barrier discharge over liquid covered tissue, 5000 voltage pulses were simulated, followed by 5 min of afterglow. Due to the accumulation of long-lived species such as ozone and N x O y , the gas phase dynamics of the 5000th discharge pulse are different from those of the first pulse, particularly with regards to the negative ions. The consequences of applied voltage, gas flow, pulse repetition frequency, and the presence of organic molecules in the liquid on the gas and liquid reactive species are discussed.

Waveguiding and bending modes in a plasma photonic crystal bandgap device

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang, B., E-mail: bwang17@stanford.edu; Cappelli, M. A.

2016-06-15

Waveguiding and bending modes are investigated in a fully tunable plasma photonic crystal. The plasma device actively controls the propagation of free space electromagnetic waves in the S to X band of the microwave spectrum. An array of discharge plasma tubes form a square crystal lattice exhibiting a well-defined bandgap, with individual active switching of the plasma elements to allow for waveguiding and bending modes to be generated dynamically. We show, through simulations and experiments, the existence of transverse electric (TE) mode waveguiding and bending modes.

A dc non-thermal atmospheric-pressure plasma microjet

NASA Astrophysics Data System (ADS)

Zhu, WeiDong; Lopez, Jose L.

2012-06-01

A direct current (dc), non-thermal, atmospheric-pressure plasma microjet is generated with helium/oxygen gas mixture as working gas. The electrical property is characterized as a function of the oxygen concentration and show distinctive regions of operation. Side-on images of the jet were taken to analyze the mode of operation as well as the jet length. A self-pulsed mode is observed before the transition of the discharge to normal glow mode. Optical emission spectroscopy is employed from both end-on and side-on along the jet to analyze the reactive species generated in the plasma. Line emissions from atomic oxygen (at 777.4 nm) and helium (at 706.5 nm) were studied with respect to the oxygen volume percentage in the working gas, flow rate and discharge current. Optical emission intensities of Cu and OH are found to depend heavily on the oxygen concentration in the working gas. Ozone concentration measured in a semi-confined zone in front of the plasma jet is found to be from tens to ˜120 ppm. The results presented here demonstrate potential pathways for the adjustment and tuning of various plasma parameters such as reactive species selectivity and quantities or even ultraviolet emission intensities manipulation in an atmospheric-pressure non-thermal plasma source. The possibilities of fine tuning these plasma species allows for enhanced applications in health and medical related areas.

A Numerical Study of the Non-Ideal Behavior, Parameters, and Novel Applications of an Electrothermal Plasma Source

NASA Astrophysics Data System (ADS)

Winfrey, A. Leigh

Electrothermal plasma sources have numerous applications including hypervelocity launchers, fusion reactor pellet injection, and space propulsion systems. The time evolution of important plasma parameters at the source exit is important in determining the suitability of the source for different applications. In this study a capillary discharge code has been modified to incorporate non-ideal behavior by using an exact analytical model for the Coulomb logarithm in the plasma electrical conductivity formula. Actual discharge currents from electrothermal plasma experiments were used and code results for both ideal and non-ideal plasma models were compared to experimental data, specifically the ablated mass from the capillary and the electrical conductivity as measured by the discharge current and the voltage. Electrothermal plasma sources operating in the ablation-controlled arc regime use discharge currents with pulse lengths between 100 micros to 1 ms. Faster or longer or extended flat-top pulses can also be generated to satisfy various applications of ET sources. Extension of the peak current for up to an additional 1000 micros was tested. Calculations for non-ideal and ideal plasma models show that extended flattop pulses produce more ablated mass, which scales linearly with increased pulse length while other parameters remain almost constant. A new configuration of the PIPE source has been proposed in order to investigate the formation of plasmas from mixed materials. The electrothermal segmented plasma source can be used for studies related to surface coatings, surface modification, ion implantation, materials synthesis, and the physics of complex mixed plasmas. This source is a capillary discharge where the ablation liner is made from segments of different materials instead of a single sleeve. This system should allow for the modeling and characterization of the growth plasma as it provides all materials needed for fabrication through the same method. An ablation-free capillary discharge computer code has been developed to model plasma flow and acceleration of pellets for fusion fueling in magnetic fusion reactors. Two case studies with and without ablation, including different source configurations have been studied here. Velocities necessary for fusion fueling have been achieved. New additions made to the code model incorporate radial heat and energy transfer and move ETFLOW towards being a 2-D model of the plasma flow. This semi 2-D approach gives a view of the behavior of the plasma inside the capillary as it is affected by important physical parameters such as radial thermal heat conduction and their effect on wall ablation.

Spectroscopic investigation of a dielectric barrier discharge in modified atmosphere packaging

NASA Astrophysics Data System (ADS)

Milosavljević, Vladimir; Cullen, Patrick J.

2017-11-01

Diagnostics of a dielectric barrier discharge (DBD), in a sealed package (with and without meat) filled with gas mixtures of oxygen and carbon-dioxide (O2-CO2), is reported. The generation and evaluation of the plasma chemistry induced within the confines of the sealed package is studied. The plasma discharges were analyzed by optical emission spectroscopy (OES) and optical absorption spectroscopy (OAS) over a range of plasma process parameters. The study includes a detailed experimental investigation of the spatial and temporal spectroscopic data and links them with plasma kinetics. The results from the spectral radiation from package provide information about the electron energy distribution function. The experimental data indicates that the humidity level in the package with and without meat is unchanged, and that the gas temperature was not significantly modified. Oxygen and nitrogen radicals (trapped gas atmosphere and modified atmosphere) are increased in the package containing meat; at the same time there is no evidence of the presence of carbon monoxide molecules. The role of the nitrogen molecule in the quenching of O2 and CO2 molecules is also evaluated.

The quenching effect of hydrogen on the nitrogen in metastable state in atmospheric-pressure N{sub 2}-H{sub 2} microwave plasma torch

DOE Office of Scientific and Technical Information (OSTI.GOV)

Li, Shou-Zhe, E-mail: lisz@dlut.edu.cn; Zhang, Xin; Chen, Chuan-Jie

2014-07-15

The atmospheric-pressure microwave N{sub 2}-H{sub 2} plasma torch is generated and diagnosed by optical emission spectroscopy. It is found that a large amount of N atoms and NH radicals are generated in the plasma torch and the emission intensity of N{sub 2}{sup +} first negative band is the strongest over the spectra. The mixture of hydrogen in nitrogen plasma torch causes the morphology of the plasma discharge to change with appearance that the afterglow shrinks greatly and the emission intensity of N{sub 2}{sup +} first negative band decreases with more hydrogen mixed into nitrogen plasma. In atmospheric-pressure microwave-induced plasma torch,more » the hydrogen imposes a great influence on the characteristics of nitrogen plasma through the quenching effect of the hydrogen on the metastable state of N{sub 2}.« less

Decomposition of acetaminophen in water by a gas phase dielectric barrier discharge plasma combined with TiO2-rGO nanocomposite: Mechanism and degradation pathway.

PubMed

Zhang, Guyu; Sun, Yabing; Zhang, Chunxiao; Yu, Zhongqing

2017-02-05

Acetaminophen (APAP) served as the model pollutant to evaluate the feasibility of pollutant removal by gas phase dielectric barrier discharge plasma combined with the titanium dioxide-reduced Graphene Oxide (TiO 2 -rGO) nanocomposite. TiO 2 -rGO nanocomposite was prepared using the modified hydrothermal method and characterized by TEM and XPS before and after plasma process. The results indicated that the APAP degradation efficiency was significantly improved to 92% after 18min of discharge plasma treatment coupling 0.25gL -1 TiO 2 -rGO 5%wt at 18kV, compared with the plasma alone and plasma combined with P25 TiO 2 . The degradation mechanism for APAP in this system was studied by investigating the effects of the operational variables (e.g. discharge voltage and pH value) and the amount of the generated active species; and the results showed that O 3 and H 2 O 2 yields were influenced notably by adding TiO 2 -rGO. Also, it was observed that, compared with unused TiO 2 -rGO, the photocatalytic performance of used TiO 2 -rGO declined after several recirculation times due to the further reduction of Graphene Oxide in plasma system. Finally, intermediate products were analyzed by UV-vis spectrometry and HPLC/MS, and possible transformation pathways were identified with the support of theoretically calculating the frontier electron density of APAP. Copyright © 2016 Elsevier B.V. All rights reserved.

Estimation of the ionic charge of non-metallic species into an electrical discharge through a web application

NASA Astrophysics Data System (ADS)

Pérez Gutiérrez, B. R.; Vera-Rivera, F. H.; Niño, E. D. V.

2016-08-01

Estimate the ionic charge generated in electrical discharges will allow us to know more accurately the concentration of ions implanted on the surfaces of nonmetallic solids. For this reason, in this research a web application was developed to allow us to calculate the ionic charge generated in an electrical discharge from the experimental parameters established in an ion implantation process performed in the JUPITER (Joint Universal Plasma and Ion Technologies Experimental Reactor) reactor. The estimated value of the ionic charge will be determined from data acquired on an oscilloscope, during startup and shutdown of electrical discharge, which will then be analyzed and processed. The study will provide best developments with regard to the application of ion implantation in various industrial sectors.

Gene Transfection Method Using Atmospheric Pressure Dielectric-Barrier Discharge Plasmas

NASA Astrophysics Data System (ADS)

Sasaki, Shota; Kanzaki, Makoto; Kaneko, Toshiro

2013-09-01

Gene transfection which is the process of deliberately introducing nucleic acids into cells is expected to play an important role in medical treatment because the process is necessary for gene therapy and creation of induced pluripotent stem (iPS) cells. However, the conventional transfection methods have some problems, so we focus attention on promising transfection methods by atmospheric pressure dielectric-barrier discharge (AP-DBD) plasmas. AP-DBD He plasmas are irradiated to the living cell covered with genes. Preliminarily, we use fluorescent dye YOYO-1 instead of the genes and use LIVE/DEAD Stain for cell viability test, and we analyze the transfection efficiency and cell viability under the various conditions. It is clarified that the transfection efficiency is strongly dependence on the plasma irradiation time and cell viability rates is high rates (>90%) regardless of long plasma irradiation time. These results suggest that ROS (Reactive Oxygen Species) and electric field generated by the plasma affect the gene transfection. In addition to this (the plasma irradiation time) dependency, we now investigate the effect of the plasma irradiation under the various conditions.

Effect of atmospheric pressure dielectric barrier discharge plasma on the biological activity of naringin.

PubMed

Kim, Hyun-Joo; Yong, Hae In; Park, Sanghoo; Kim, Kijung; Kim, Tae Hoon; Choe, Wonho; Jo, Cheorun

2014-10-01

The biological activity of naringin treated with atmospheric pressure plasma was evaluated to investigate whether exposure to plasma can be used as a method to improve the biological activity of natural materials. Naringin was dissolved in methanol (at 500 ppm) and transferred to a container. A dielectric barrier discharge (DBD) (250 W, 15 kHz, ambient air) was then generated. Treatment with the plasma for 20 min increased the radical-scavenging activity, FRAP value, and the total phenolic compound content of naringin from 1.45% to 38.20%, from 27.78 to 207.78 μM/g, and from 172.50 to 225.83 ppm, respectively. Moreover, the tyrosinase-inhibition effect of naringin increased from 6.12% to 83.30% upon plasma treatment. Naringin treated with plasma exhibited antimicrobial activity against foodborne pathogens, especially Salmonella Typhimurium; an activity that was absent before plasma treatment. Structural modifications induced in the naringin molecule by plasma might be responsible for improving the biological activity of naringin. Copyright © 2014 Elsevier Ltd. All rights reserved.

Hierarchical modeling of plasma and transport phenomena in a dielectric barrier discharge reactor

NASA Astrophysics Data System (ADS)

Bali, N.; Aggelopoulos, C. A.; Skouras, E. D.; Tsakiroglou, C. D.; Burganos, V. N.

2017-12-01

A novel dual-time hierarchical approach is developed to link the plasma process to macroscopic transport phenomena in the interior of a dielectric barrier discharge (DBD) reactor that has been used for soil remediation (Aggelopoulos et al 2016 Chem. Eng. J. 301 353-61). The generation of active species by plasma reactions is simulated at the microseconds (µs) timescale, whereas convection and thermal conduction are simulated at the macroscopic (minutes) timescale. This hierarchical model is implemented in order to investigate the influence of the plasma DBD process on the transport and reaction mechanisms during remediation of polluted soil. In the microscopic model, the variables of interest include the plasma-induced reactive concentrations, while in the macroscopic approach, the temperature distribution, and the velocity field both inside the discharge gap and within the polluted soil material as well. For the latter model, the Navier-Stokes and Darcy Brinkman equations for the transport phenomena in the porous domain are solved numerically using a FEM software. The effective medium theory is employed to provide estimates of the effective time-evolving and three-phase transport properties in the soil sample. Model predictions considering the temporal evolution of the plasma remediation process are presented and compared with corresponding experimental data.

Fluid modeling of radical species generation mechanism in dense methane-air mixture streamer discharge

NASA Astrophysics Data System (ADS)

Qian, Muyang; Li, Gui; Kang, Jinsong; Liu, Sanqiu; Ren, Chunsheng; Zhang, Jialiang; Wang, Dezhen

2018-01-01

Atmospheric dielectric barrier discharge (DBD) was found to be promising in the context of plasma chemistry, plasma medicine, and plasma-assisted combustion. In this paper, we present a detailed fluid modeling study of abundant radical species produced by a positive streamer in atmospheric dense methane-air DBD. A two-dimensional axisymmetric fluid model is constructed, in which 82 plasma chemical reactions and 30 different species are considered. Spatial and temporal density distributions of dominant radicals and ions are presented. We lay our emphasis on the effect of varying relative permittivity (ɛr = 2, 4.5, and 9) on the streamer dynamics in the plasma column, such as electric field behavior, production, and destruction pathways of dominant radical species. We find that higher relative permittivity promotes propagation of electric field and formation of conduction channel in the plasma column. The streamer discharge is sustained by the direct electron-impact ionization of methane molecule. Furthermore, the electron-impact dissociation of methane (e + CH4 = >e + H+CH3) is found to be the dominant reaction pathway to produce CH3 and H radicals. Similarly, the electron-impact dissociations of oxygen (e + O2 = >e + O+O(1D), e + O2 = >e + O+O) are the major routes for O production.

Study of Pulsed vs. RF Plasma Properties for Surface Processing Applications

NASA Astrophysics Data System (ADS)

Tang, Ricky; Hopkins, Matthew; Barnat, Edward; Miller, Paul

2015-09-01

The ability to manipulate the plasma parameters (density, E/N) was previously demonstrated using a double-pulsed column discharge. Experiments extending this to large-surface plasmas of interest to the plasma processing community were conducted. Differences between an audio-frequency pulsed plasma and a radio-frequency (rf) discharge, both prevalent in plasma processing applications, were studied. Optical emission spectroscopy shows higher-intensity emission in the UV/visible range for the pulsed plasma comparing to the rf plasma at comparable powers. Data suggest that the electron energy is higher for the pulsed plasma leading to higher ionization, resulting in increased ion density and ion flux. Diode laser absorption measurements of the concentration of the 1S5 metastable and 1S4 resonance states of argon (correlated with the plasma E/N) provide comparisons between the excitation/ionization states of the two plasmas. Preliminary modeling efforts suggest that the low-frequency polarity switch causes a much more abrupt potential variation to support interesting transport phenomena, generating a ``wave'' of higher temperature electrons leading to more ionization, as well as ``sheath capture'' of a higher density bolus of ions that are then accelerated during polarity switch.

Effect of nitrogen addition to ozone generation characteristics by diffuse and filamentary dielectric barrier discharges at atmospheric pressure

NASA Astrophysics Data System (ADS)

Osawa, Naoki; Tsuji, Takafumi; Ogiso, Ryota; Yoshioka, Yoshio

2017-05-01

Ozone is widely used for gas treatment, advanced oxidation processes, microorganisms inactivation, etc. In this research, we investigated the effect of nitrogen addition to ozone generation characteristics by atmospheric pressure Townsend discharge (APTD) type and filamentary dielectric barrier discharge (DBD) type ozone generators. The result showed that the ozone generated by the filamentary DBD increases rapidly with the increase of O2 content, and is higher than that by the APTD. On the other hand, it is interesting that the ozone generated by the APTD gradually decreases with the increase of O2 content. In order to clarify why the characteristics of ozone generation by the two kinds of discharge modes showed different dependency to the N2 content, we analyzed the exhaust gas composition using FTIR spectroscopy and calculated the rate coefficients using BOLSIG+ code. As a result, we found that although O2 content decreased with increasing N2 content, additional O atoms produced by excited N2 molecules contribute to ozone generation in case of APTD. Contribution to the topical issue "The 15th International Symposium on High Pressure Low Temperature Plasma Chemistry (HAKONE XV)", edited by Nicolas Gherardi and Tomáš Hoder

23RD International Conference on Phenomena in Ionized Gases, Volume 5

DTIC Science & Technology

1998-12-01

eNm.f, generated within the plasma is given by section with a 5-cm diameter. The magnetic field was Vof = wh Bt p i vn provided by an iron- core ...cylindrical tungsten probes, of 0.038cm. as impurities can be centrifuged as reported by diameter, insulated by thin glass tube except their tips Bonnevier...Norfolk, VA 213529 1. Discharge modes discharge begins, at several hundred Torr, to change from a hollow cathode discharge into what we Experimental

Discharge source with gas curtain for protecting optics from particles

DOEpatents

Fornaciari, Neal R.; Kanouff, Michael P.

2004-03-30

A gas curtain device is employed to deflect debris that is generated by an extreme ultraviolet and soft x-ray radiation discharge source such as an electric discharge plasma source. The gas curtain device projects a stream of gas over the path of the radiation to deflect debris particles into a direction that is different from that of the path of the radiation. The gas curtain can be employed to prevent debris accumulation on the optics used in photolithography.

Measurements of Electric Field in a Nanosecond Pulse Discharge by 4-WAVE Mixing

NASA Astrophysics Data System (ADS)

Baratte, Edmond; Adamovich, Igor V.; Simeni Simeni, Marien; Frederickson, Kraig

2017-06-01

Picosecond four-wave mixing is used to measure temporally and Picosecond four-wave mixing is used to measure temporally and spatially resolved electric field in a nanosecond pulse dielectric discharge sustained in room air and in an atmospheric pressure hydrogen diffusion flame. Measurements of the electric field, and more precisely the reduced electric field (E/N) in the plasma is critical for determination rate coefficients of electron impact processes in the plasma, as well as for quantifying energy partition in the electric discharge among different molecular energy modes. The four-wave mixing measurements are performed using a collinear phase matching geometry, with nitrogen used as the probe species, at temporal resolution of about 2 ns . Absolute calibration is performed by measurement of a known electrostatic electric field. In the present experiments, the discharge is sustained between two stainless steel plate electrodes, each placed in a quartz sleeve, which greatly improves plasma uniformity. Our previous measurements of electric field in a nanosecond pulse dielectric barrier discharge by picosecond 4-wave mixing have been done in air at room temperature, in a discharge sustained between a razor edge high-voltage electrode and a plane grounded electrode (a quartz plate or a layer of distilled water). Electric field measurements in a flame, which is a high-temperature environment, are more challenging because the four-wave mixing signal is proportional to the to square root of the difference betwen the populations of N2 ground vibrational level (v=0) and first excited vibrational level (v=1). At high temperatures, the total number density is reduced, thus reducing absolute vibrational level populations of N2. Also, the signal is reduced further due to a wider distribution of N2 molecules over multiple rotational levels at higher temperatures, while the present four-wave mixing diagnostics is using spectrally narrow output of a ps laser and a high-pressure Raman cell, providing access only to a few N2 rotational levels. Because of this, the four-wave mixing signal in the flame is lower by more than an order of magnitude compared to the signal generated in room temperature air plasma. Preliminary experiments demonstrated four-wave mixing signal generated by the electric field in the flame, following ns pulse discharge breakdown. The electric field in the flame is estimated using four-wave mixing signal calibration vs. temperature in electrostatic electric field generated in heated air. Further measurements in the flame are underway.

Model of the Streamer Zone of a Leader

NASA Astrophysics Data System (ADS)

Milikh, G. M.; Raina, A.; Shneider, M.; Likhanskii, A.; George, A.

2015-12-01

Developed leaders represent highly conductive plasma channels, continuously emitting a fan of streamers, termed the streamer zone. The tip moves at a speed much slower than that of individual streamers. A huge number of short-lived streamers in the corona generate the space charge field required to maintain the streamer propagation. A critical issue is the conversion from the streamer to leader phase [Da Silva and Pasko, 2013]. The objective of this paper is to present simulations of the formation and propagation of the streamer zone of a leader. In these simulations we generated a group of streamers that propagate in a discharge gap while they interact with each other. We use the modified numerical model [Likhanskii et al., 2007] developed to simulate discharge plasma actuators driven by nanosecond pulses. The model uses 2D rectangular computational box, and the discharge gap is filled with the air at normal conditions. Furthermore the model considers electrons, positive and negative ions. The plasma kinetics and interaction with neutral molecules is modeled in a drift-diffusion approximation [Likhanskii et al., 2007]. The electric field and potential are related to the density of charged species according to the Poisson equation. The latter was solved by the successive over-relaxation method. It is shown that interaction between the streamers significantly reduces their propagation velocity. Furthermore the streamer velocity depends on the distance between the streamers. The smaller is that distance the stronger is the suppression of the streamer velocity. This explains why the leader, which consists of many streamers, is much slower than a single streamer formed in the same discharge gap. C.L. Da Silva and V.P. Pasko, J. Geophys. Res.: Atmospheres, 118, 1-30, 2013 A.V. Likhanskii et al., Phys. Plasmas, 14, 073501, 2007.

Measurement of activated species generated by AC power excited non-equilibrium atmospheric pressure Ar plasma jet with air engulfment

NASA Astrophysics Data System (ADS)

Takeda, Keigo; Ishikawa, Kenji; Tanaka, Hiromasa; Kano, Hiroyuki; Sekine, Makoto; Hori, Masaru

2013-09-01

Non-equilibrium atmospheric pressure plasma jet (NEAPPJ) is very attractive tool for bio and medical applications. In the plasma treatments, samples are typically located at a far region from main discharge, and treated in open air without purge gases. Influence of air engulfment on generation of activated species in the NEAPPJ in open air is a large issue for the application. In this study, the AC excited argon NEAPPJ with the gas flow rate of 2 slm was generated under the open air condition. The densities of the grand state nitrogen monoxide (NO) and the ground state O atom generated by the NEAPPJ were measured by laser induced fluorescence spectroscopy and vacuum ultraviolet absorption spectroscopy. The length of the plasma jet was around 10 mm. Up to 10 mm, the NO density increased with increasing the distance from plasma head, and then saturated in remote region of plasma. On the other hand, the O atom density decreased from 1014 to 1013 cm-3 with increasing the distance. Especially, the amount of decrease in O atom density became the largest at the plasma edge. We will discuss the generation and loss processes of activated species generated in the NEAPPJ with the measurement results using spectroscopic methods.

Room temperature sterilization of surfaces and fabrics with a one atmosphere uniform glow discharge plasma.

PubMed

Kelly-Wintenberg, K; Montie, T C; Brickman, C; Roth, J R; Carr, A K; Sorge, K; Wadsworth, L C; Tsai, P P

1998-01-01

We report the results of an interdisciplinary collaboration formed to assess the sterilizing capabilities of the One Atmosphere Uniform Glow Discharge Plasma (OAUGDP). This newly-invented source of glow discharge plasma (the fourth state of matter) is capable of operating at atmospheric pressure in air and other gases, and of providing antimicrobial active species to surfaces and workpieces at room temperature as judged by viable plate counts. OAUGDP exposures have reduced log numbers of bacteria, Staphylococcus aureus and Escherichia coli, and endospores from Bacillus stearothermophilus and Bacillus subtilis on seeded solid surfaces, fabrics, filter paper, and powdered culture media at room temperature. Initial experimental data showed a two-log10 CFU reduction of bacteria when 2 x 10(2) cells were seeded on filter paper. Results showed > or = 3 log10 CFU reduction when polypropylene samples seeded with E. coli (5 x 10(4)) were exposed, while a 30 s exposure time was required for similar killing with S. aureus-seeded polypropylene samples. The exposure times required to effect > or = 6 log10 CFU reduction of E. coli and S. aureus on polypropylene samples were no longer than 30 s. Experiments with seeded samples in sealed commercial sterilization bags showed little or no differences in exposure times compared to unwrapped samples. Plasma exposure times of less than 5 min generated > or = 5 log10 CFU reduction of commercially prepared Bacillus subtilis spores (1 x 10(5)); 7 min OAUGDP exposures were required to generate a > or = 3 log10 CFU reduction for Bacillus stearothermophilus spores. For all microorganisms tested, a biphasic curve was generated when the number of survivors vs time was plotted in dose-response cures. Several proposed mechanisms of killing at room temperature by the OAUGDP are discussed.

Research Activities at Plasma Research Laboratory at NASA Ames Research Center

NASA Technical Reports Server (NTRS)

Sharma, S. P.; Rao, M. V. V. S.; Meyyappan, Meyya

2000-01-01

In order to meet NASA's requirements for the rapid development and validation of future generation electronic devices as well as associated materials and processes, enabling technologies are being developed at NASA-Ames Research Center using a multi-discipline approach. The first step is to understand the basic physics of the chemical reactions in the area of plasma reactors and processes. Low pressure glow discharges are indispensable in the fabrication of microelectronic circuits. These plasmas are used to deposit materials and also etch fine features in device fabrication. However, many plasma-based processes suffer from stability and reliability problems leading to a compromise in performance and a potentially increased cost for the semiconductor manufacturing industry. Although a great deal of laboratory-scale research has been performed on many of these processing plasmas, little is known about the gas-phase and surface chemical reactions that are critical in many etch and deposition processes, and how these reactions are influenced by the variation in operating conditions. Such a lack of understanding has hindered the development of process models that can aid in the scaling and improvement of plasma etch and deposition systems. Our present research involves the study of such plasmas. An inductively-coupled plasma (ICP) source in place of the standard upper electrode assembly of the Gaseous Electronics Conference (GEC) radio-frequency (RF) Reference Cell is used to investigate the discharge characteristics. This ICP source generates plasmas with higher electron densities and lower operating pressures than obtainable with the original parallel-plate version of the GEC Cell. This expanded operating regime is more relevant to new generations of industrial plasma systems being used by the microelectronics industry. The research goal is to develop an understanding of the physical phenomena involved in plasma processing and to measure much needed fundamental parameters, such as gas phase and surface reaction rates, species concentration, temperature, ion energy distribution, and electron number density.

Optimization of the Magnetic Field Structure for Sustained Plasma Gun Helicity Injection for Magnetic Turbulence Studies at the Bryn Mawr Plasma Laboratory

NASA Astrophysics Data System (ADS)

Cartagena-Sanchez, C. A.; Schaffner, D. A.; Johnson, H. K.; Fahim, L. E.

2017-10-01

A long-pulsed magnetic coaxial plasma gun is being implemented and characterized at the Bryn Mawr Plasma Laboratory (BMPL). A cold cathode discharged between the cylindrical electrodes generates and launches plasma into a 24cm diameter, 2m long chamber. Three separately pulsed magnetic coils are carefully positioned to generate radial magnetic field between the electrodes at the gun edge in order to provide stuffing field. Magnetic helicity is continuously injected into the flux-conserving vacuum chamber in a process akin to sustained slow-formation of spheromaks. The aim of this source, however, is to supply long pulses of turbulent magnetized plasma for measurement rather than for sustained spheromak production. The work shown here details the optimization of the magnetic field structure for this sustained helicity injection.

Use of Plasma Actuators as a Moving-Wake Generator

NASA Technical Reports Server (NTRS)

Corke, Thomas C.; Thomas, Flint O.; Klapetzky Michael J.

2007-01-01

The work documented in this report tests the concept of using plasma actuators as a simple and easy way to generate a simulated moving-wake and the disturbances associated with it in turbines. This wake is caused by the blades of the upstream stages of the turbine. Two types of devices, one constructed of arrays of NACA 0018 airfoils, and the one constructed of flat plates were studied. The airfoils or plates were equipped with surface mounted dielectric barrier discharge (DBD) plasma actuators, which were used to generate flow disturbances resembling moving-wakes. CTA hot-wire anemometry and flow visualization using a smoke-wire were used to investigate the wake independence at various spacings and downstream locations. The flat plates were found to produce better results than the airfoils in creating large velocity fluctuations in the free-stream flow. Different dielectric materials, plasma actuator locations, leading edge contours, angles of attack and plate spacings were investigated, some with positive results. The magnitudes of the velocity fluctuations were found to be comparable to existing mechanical moving-wake generators, thus proving the feasibility of using plasma actuators as a moving-wake generator.

Theoretical and experimental investigation on magneto-hydrodynamics of plasma window

DOE PAGES

Wang, S. Z.; Zhu, K.; Huang, S.; ...

2016-01-05

As a new device, we designed plasma window to use plasma discharge to separate atmosphere from vacuum with high difference of pressure. It has many excellent properties, being able to be used as available passage for ion beam with negligible energy loss, also impervious to radiation damage and thermal damage. Normally beam focusing by accelerators is not that easy to achieve within channel of small cross section. 10 mm diameter plasma window's experimental realization could contribute to its further application in accelerator system. In this paper, 10 mm diameter 60 mm long plasma window has first been designed and managedmore » to generate arc discharge with argon gas experimentally. Our result proves that it has the ability to separate at least 28.8 kPa (not the upper limit) from 360 Pa with 50 A direct current and 2.5 kW power supplied. Current increase leads to linear inlet pressure increase obviously, while it has less impact on outlet pressure and voltage, coming to the conclusion that the higher current of plasma discharge, the larger pressure difference it creates. Furthermore, theoretical analysis of 10 mm diameter plasma window in axis symmetrical configuration using argon also has been provided, in which a numerical 2D FLUENT-based magneto-hydrodynamic simulation model is settled. It has a good agreement with experimental result on voltage and mass flow rate when inlet pressure is increased.« less

Estimation of optimum density and temperature for maximum efficiency of tin ions in Z discharge extreme ultraviolet sources

DOE Office of Scientific and Technical Information (OSTI.GOV)

Masnavi, Majid; Nakajima, Mitsuo; Hotta, Eiki

Extreme ultraviolet (EUV) discharge-based lamps for EUV lithography need to generate extremely high power in the narrow spectrum band of 13.5{+-}0.135 nm. A simplified collisional-radiative model and radiative transfer solution for an isotropic medium were utilized to investigate the wavelength-integrated light outputs in tin (Sn) plasma. Detailed calculations using the Hebrew University-Lawrence Livermore atomic code were employed for determination of necessary atomic data of the Sn{sup 4+} to Sn{sup 13+} charge states. The result of model is compared with experimental spectra from a Sn-based discharge-produced plasma. The analysis reveals that considerably larger efficiency compared to the so-called efficiency of amore » black-body radiator is formed for the electron density {approx_equal}10{sup 18} cm{sup -3}. For higher electron density, the spectral efficiency of Sn plasma reduces due to the saturation of resonance transitions.« less

Plasma microreactor in supercritical xenon and its application to diamondoid synthesis

NASA Astrophysics Data System (ADS)

Oshima, F.; Stauss, S.; Ishii, C.; Pai, D. Z.; Terashima, K.

2012-10-01

The generation of plasmas in a microreactor is demonstrated in xenon from atmospheric pressure up to supercritical conditions. Ac high voltage at a frequency of 15 kHz was applied across a 25-µm discharge gap between a tungsten wire and a fused silica micro-capillary tube in a coaxial configuration. Using this continuous flow supercritical fluid microreactor, it was possible to synthesize diamantane and other diamondoids up to nonamantane, using adamantane as a precursor and seed. It is anticipated that plasmas generated in supercritical fluid microreactors may not only allow faster fabrication of diamondoids, but also offer opportunities for the fabrication of other nanomaterials.

The development and application of a cold atmospheric plasma generator for treatment of skin and soft-tissue injuries in animals

NASA Astrophysics Data System (ADS)

Emelyanov, O. A.; Petrova, N. O.; Smirnova, N. V.; Shemet, M. V.

2017-08-01

We describe a device for obtaining cold plasma in air at atmospheric pressure using a system of positive high-voltage pin electrodes, which is intended for the treatment of skin and soft-tissue injuries in animals. Plasma is generated due to the development of periodic pulsed discharge of nanosecond duration at current pulse amplitudes 10-20 mA, characteristic frequencies 10-20 kHz, and applied voltages within 8-10 kV. The high efficacy of the proposed device and method is confirmed by the good clinical results of treating large domestic animals with traumatic injuries.

Experimentally Determined Plasma Parameters in a 30 cm Ion Engine

NASA Technical Reports Server (NTRS)

Sengupta, Anita; Goebel, Dan; Fitzgerald, Dennis; Owens, Al; Tynan, George; Dorner, Russ

2004-01-01

Single planar Langmuir probes and fiber optic probes are used to concurrently measure the plasma properties and neutral density variation in a 30cm diameter ion engine discharge chamber, from the immediate vicinity of the keeper to the near grid plasma region. The fiber optic probe consists of a collimated optical fiber recessed into a double bore ceramic tube fitted with a stainless steel light-limiting window. The optical fiber probe is used to measure the emission intensity of excited neutral xenon for a small volume of plasma, at various radial and axial locations. The single Langmuir probes, are used to generate current-voltage characteristics at a total of 140 spatial locations inside the discharge chamber. Assuming a maxwellian distribution for the electron population, the Langmuir probe traces provide spatially resolved measurements of plasma potential, electron temperature, and plasma density. Data reduction for the NSTAR TH8 and TH15 throttle points indicates an electron temperature range of 1 to 7.9 eV and an electron density range of 4e10 to le13 cm(sup -3), throughout the discharge chamber, consistent with the results in the literature. Plasma potential estimates, computed from the first derivative of the probe characteristic, indicate potential from 0.5V to 11V above the discharge voltage along the thruster centerline. These values are believed to be excessively high due to the sampling of the primary electron population along the thruster centerline. Relative neutral density profiles are also obtained with a fiber optic probe sampling photon flux from the 823.1 nm excited to ground state transition. Plasma parameter measurements and neutral density profiles will be presented as a function of probe location and engine discharge conditions. A discussion of the measured electron energy distribution function will also be presented, with regards to variation from pure maxwellian. It has been found that there is a distinct primary population found along the thruster centerline, which causes estimates of electron temperature, electron density, and plasma potential, to err on the high side, due this energetic population. Computation of the energy distribution fimction of the plasma clearly indicates the presence of primaries, whose presence become less obvious with radial distance from the main discharge plume.

Cathode luminescence light source for broadband applications in the visible spectrum

NASA Technical Reports Server (NTRS)

Foster, John E. (Inventor)

2007-01-01

A device and method for generating cathode luminescence is provided. The device and method generate broad spectrum electromagnetic radiation in the visible. A layer of particles, such as quartz or alumina powder, is exposed to electrons in a plasma discharge. Surface excitation of these particles or the generations/excitation of F-center sites give rise to luminescence.

Effect of Si on DC arc plasma generation from Al-Cr and Al-Cr-Si cathodes used in oxygen

NASA Astrophysics Data System (ADS)

Zhirkov, I.; Landälv, L.; Göthelid, E.; Ahlgren, M.; Eklund, P.; Rosen, J.

2017-02-01

Al2O3 alloyed with Cr is an important material for the tooling industry. It can be synthesized from an arc discharge using Al-Cr cathodes in an oxygen atmosphere. Due to formation of Al-rich oxide islands on the cathode surface, the arc process stability is highly sensitive to oxygen pressure. For improved stability, the use of Al0.70Cr0.25Si0.05 cathodes has previously been suggested, where Si may reduce island formation. Here, we have investigated the effect of Si by comparing plasma generation and thin film deposition from Al0.7Cr0.3 and Al0.7Cr0.25Si0.05 cathodes. Plasma ion composition, ion energies, ion charge states, neutral species, droplet formation, and film composition have been characterized at different O2 flow rates for arc currents of 60 and 90 A. Si and related compounds are detected in plasma ions and in plasma neutrals. Scanning electron microscopy and energy dispersive X-ray analysis show that the cathode composition and the film composition are the same, with Si present in droplets as well. The effect of Si on the process stability, ion energies, and ion charge states is found to be negligible compared to that of the arc current. The latter is identified as the most relevant parameter for tuning the properties of the reactive discharge. The present work increases the fundamental understanding of plasma generation in a reactive atmosphere, and provides input for the choice of cathode composition and process parameters in reactive DC arc synthesis.

Beam-plasma instabilities and the beam-plasma discharge

NASA Technical Reports Server (NTRS)

Kellogg, P. J.; Boswell, R. W.

1986-01-01

Using a new waves on magnetized beams and turbulence (WOMBAT) 0-450 eV electron gun, measurements bearing on the generation of beam-plasma discharge (BPD) are made. The new gun has a narrower divergence angle than the old, and the BPD ignition current is found to be proportional to the cross-sectional area of the plasma. The high-frequency instabilities are identified with the two Trivelpiece-Gould modes, (1959). The upper frequency is identified as a Cerenkov resonance with the upper Trivelpiece-Gould mode, and the lower frequency with a cyclotron resonance with the lower mode, in agreement with theoretical expectations. Convective growth rates are found to be small. A mechanism involving the conversion of a convective instability to an absolute one by trapping of the unstable waves in the density perturbations of the low-frequency waves, is suggested for the low-frequency wave control of the onset of the high frequency precursors to the BPD.

Paraelectric gas flow accelerator

NASA Technical Reports Server (NTRS)

Sherman, Daniel M. (Inventor); Wilkinson, Stephen P. (Inventor); Roth, J. Reece (Inventor)

2001-01-01

A substrate is configured with first and second sets of electrodes, where the second set of electrodes is positioned asymmetrically between the first set of electrodes. When a RF voltage is applied to the electrodes sufficient to generate a discharge plasma (e.g., a one-atmosphere uniform glow discharge plasma) in the gas adjacent to the substrate, the asymmetry in the electrode configuration results in force being applied to the active species in the plasma and in turn to the neutral background gas. Depending on the relative orientation of the electrodes to the gas, the present invention can be used to accelerate or decelerate the gas. The present invention has many potential applications, including increasing or decreasing aerodynamic drag or turbulence, and controlling the flow of active and/or neutral species for such uses as flow separation, altering heat flow, plasma cleaning, sterilization, deposition, etching, or alteration in wettability, printability, and/or adhesion.

Effect of a direct current bias on the electrohydrodynamic performance of a surface dielectric barrier discharge actuator for airflow control

NASA Astrophysics Data System (ADS)

Yan, Huijie; Yang, Liang; Qi, Xiaohua; Ren, Chunsheng

2015-02-01

The effect of a DC bias on the electrohydrodynamics (EHD) force induced by a surface dielectric barrier AC discharge actuator for airflow control at the atmospheric pressure is investigated. The measurement of the surface potential due to charge deposition at different DC biases is carried out by using a special designed corona like discharge potential probe. From the surface potential data, the plasma electromotive force is shown not affected much by the DC biases except for some reduction of the DC bias near the exposed electrode edge for the sheath-like configuration. The total thrust is measured by an analytical balance, and an almost linear relationship to the potential voltage at the exposed electrode edge is found for the direct thrust force. The temporally averaged ionic wind characteristics are investigated by Pitot tube sensor and schlieren visualization system. It is found that the ionic wind velocity profiles with different DC biases are almost the same in the AC discharge plasma area but gradually diversified in the further downstream area as well as the upper space away from the discharge plasma area. Also, the DC bias can significantly modify the topology of the ionic wind produced by the AC discharge actuator. These results can provide an insight into how the DC biases to affect the force generation.

Effects of dielectric barrier discharge plasma on the inactivation of Zygosaccharomyces rouxii and quality of apple juice.

PubMed

Xiang, Qisen; Liu, Xiufang; Li, Junguang; Liu, Shengnan; Zhang, Hua; Bai, Yanhong

2018-07-15

This work aimed to evaluate the effects of dielectric barrier discharge (DBD) plasma on inactivation of spoilage yeast Zygosaccharomyces rouxii (Z. rouxii), in apple juice. Results showed that DBD plasma treatment at 90 W for 140 s resulted in about 5-log reduction of Z. rouxii in apple juice. The levels of extracellular nucleic acids and proteins as well as contents of H 2 O 2 and NO 2 - in yeast extract-peptone-dextrose (YPD) medium increased significantly after DBD plasma treatment at 90 W for 40-200 s. The increases in membrane permeability and generation of reactive species would likely contribute to DBD plasma-mediated inactivation of Z. rouxii. DBD plasma caused significant changes in pH, titratable acidity, and certain color parameters of apple juice, but had no effect on the contents of total soluble solids, reducing sugar, and total phenolics. This study provides key implications for the application of DBD plasma in fruit juice processing. Copyright © 2018 Elsevier Ltd. All rights reserved.

Characteristics of the inductive nitrogen laser generation

NASA Astrophysics Data System (ADS)

Razhev, A. M.; Churkin, D. S.; Kargapoltsev, E. S.

2016-05-01

The results of the experimental study of energy, temporal, spectral and spatial characteristics of UV inductive laser generation are presented. The study has identified a number of characteristics which demonstrate the differences between electron parameters of inductively coupled plasma and the plasma of longitudinal and transverse electrical discharges. The mechanism of simultaneous occurrence of Lewis-Rayleigh afterglow representing transitions between higher vibrational substates of B3Πg and A3∑u+ states; laser generation at C3Πu→B3Πg transition as well as the absence of IR radiation at 1st positive system typical for electrical discharge nitrogen lasers has been thoroughly researched. The major characteristic is ring shaped laser beam which size and width depend on excitation conditions. Inductive UV nitrogen laser is found to operate in ASE regime, but has a low divergence of 0.4±0.1 mrad and high pulse-to-pulse stability (laser pulse deviation amplitude did not exceed 1%).

Effects of oxygen concentration on atmospheric pressure dielectric barrier discharge in Argon-Oxygen Mixture

NASA Astrophysics Data System (ADS)

Li, Xuechun; Li, Dian; Wang, Younian

2016-09-01

A dielectric barrier discharge (DBD) can generate a low-temperature plasma easily at atmospheric pressure and has been investigated for applications in trials in cancer therapy, sterilization, air pollution control, etc. It has been confirmed that reactive oxygen species (ROS) play a key role in the processes. In this work, we use a fluid model to simulate the plasma characteristics for DBD in argon-oxygen mixture. The effects of oxygen concentration on the plasma characteristics have been discussed. The evolution mechanism of ROS has been systematically analyzed. It was found that the ground state oxygen atoms and oxygen molecular ions are the dominated oxygen species under the considered oxygen concentrations. With the oxygen concentration increasing, the densities of electrons, argon atomic ions, resonance state argon atoms, metastable state argon atoms and excited state argon atoms all show a trend of decline. The oxygen molecular ions density is high and little influenced by the oxygen concentration. Ground state oxygen atoms density tends to increase before falling. The ozone density increases significantly. Increasing the oxygen concentration, the discharge mode begins to change gradually from the glow discharge mode to Townsend discharge mode. Project supported by the National Natural Science Foundation of China (Grant No. 11175034).

Evolution of Spatial pH Distribution in Aqueous Solution induced by Atmospheric Pressure Plasma

NASA Astrophysics Data System (ADS)

Takahashi, Shigenori; Mano, Kakeru; Hayashi, Yui; Takada, Noriharu; Kanda, Hideki; Goto, Motonobu

2016-09-01

Discharge plasma at gas-liquid interface produces some active species, and then they affect chemical reactions in aqueous solution, where pH of aqueous solution is changed due to redox species. The pH change of aqueous solution is an important factor for chemical reactions. However, spatial pH distribution in a reactor during the discharge has not been clarified yet. Thus, this work focused on spatial pH distribution of aqueous solution when pulsed discharge plasma was generated from a copper electrode in gas phase to aqueous solution in a reactor. Experiments were conducted using positive unipolar pulsed power. The unipolar pulsed voltage at +8.0 kV was applied to the copper electrode and the bottom of the reactor was grounded. The size of the reactor was 80 mm wide, 10 mm deep, and 40 mm high. The electrode was set at distance of 2 mm from the solution surface. Anthocyanins were contained in the aqueous solution as a pH indicator. The change pH solution spread horizontally, and low pH region of 10 mm in depth was formed. After discharge for 10 minutes, the low pH region was diffused toward the bottom of the reactor. After discharge for 60 minutes, the pH of the whole solution decreased.

Collective acceleration of laser plasma in a nonstationary and nonuniform magnetic field

NASA Astrophysics Data System (ADS)

Isaev, A.; Kozlovskiy, K.; Shikanov, A.; Vovchenko, E.

2017-12-01

This paper presents the new experimental results concerning acceleration of deuterium ions extracted from laser plasma in the rapid-growing nonuniform magnetic field in order to initiate the nuclear reactions D(d, n)3He and T(d, n)4He. For obtaining of laser plasma a Nd: YAG laser (λ = 1,06 μm) that generates in Q-switched mode the radiation pulses with the energy W ≤ 0,85 J and duration of τ ≈ 10 ns was used. Rapid-growing magnetic field was created with the discharge of Arkadyev-Marx pulsed-voltage generator to conical coil with the inductance of 0,65 μΗ. At characteristic discharge time of 30 ns, the rate of magnetic field growth achieved 2·107 T/s. Ion velocity was determined with the time-of-flight technique. During the experiment on deuterium plasma an ion flux velocity of ∼3 · 108 cm/s was obtained, which corresponds to the deuteron energy of ∼100 keV. Herewith, for target power density of ∼5·1011 W/cm2 obtaining of up to 1015 of accelerated deuterons and up to 108 of neutrons per a pulse is expected.

Pulsed-plasma gas-discharge inactivation of microbial pathogens in chilled poultry wash water.

PubMed

Rowan, N J; Espie, S; Harrower, J; Anderson, J G; Marsili, L; MacGregor, S J

2007-12-01

A pulsed-plasma gas-discharge (PPGD) system was developed for the novel decontamination of chilled poultry wash water. Treatment of poultry wash water in the plasma generation chamber for up to 24 s at 4 degrees C reduced Escherichia coli NCTC 9001, Campylobacter jejuni ATCC 33560, Campylobacter coli ATCC 33559, Listeria monocytogenes NCTC 9863, Salmonella enterica serovar Enteritidis ATCC 4931, and S. enterica serovar Typhimurium ATCC 14028 populations to non-detectable levels (< or = 8 log CFU/ml). Although similar PPGD treatments at 4 degrees C also produced significant reductions (> or = 3 log CFU/ml) in recalcitrant B. cereus NCTC 11145 endospore numbers within 30 s, the level of endospore reduction was dependent on the nature of the sparged gas used in the plasma treatments. Scanning electron microscopy revealed that significant damage occurred at the cellular level in PPGD-treated test organisms. This electrotechnology delivers energy in intense ultrashort bursts, generating products such as ozone, UV light, acoustic and shock waves, and pulsed electric fields that have multiple bactericidal properties. This technology offers an exciting complementary or alternative approach for treating raw poultry wash water and for preventing cross-contamination in processing environments.

Towards higher stability of resonant absorption measurements in pulsed plasmas.

PubMed

Britun, Nikolay; Michiels, Matthieu; Snyders, Rony

2015-12-01

Possible ways to increase the reliability of time-resolved particle density measurements in pulsed gaseous discharges using resonant absorption spectroscopy are proposed. A special synchronization, called "dynamic source triggering," between a gated detector and two pulsed discharges, one representing the discharge of interest and another being used as a reference source, is developed. An internal digital delay generator in the intensified charge coupled device camera, used at the same time as a detector, is utilized for this purpose. According to the proposed scheme, the light pulses from the reference source follow the gates of detector, passing through the discharge of interest only when necessary. This allows for the utilization of short-pulse plasmas as reference sources, which is critical for time-resolved absorption analysis of strongly emitting pulsed discharges. In addition to dynamic source triggering, the reliability of absorption measurements can be further increased using simultaneous detection of spectra relevant for absorption method, which is also demonstrated in this work. The proposed methods are illustrated by the time-resolved measurements of the metal atom density in a high-power impulse magnetron sputtering (HiPIMS) discharge, using either a hollow cathode lamp or another HiPIMS discharge as a pulsed reference source.

Sterilization of medical equipment and contaminated articles by making use of a resistive barrier discharge

NASA Astrophysics Data System (ADS)

Uhm, Han S.; Kang, Jung G.; Choi, Eun H.; Cho, Guang S.

2012-08-01

Presented here is an apparatus consisting of an atmospheric resistive-barrier discharge for the sterilization of medical tools wrapped in typical hospital cloths, for the sterilization of manufactured drugs in typical packaging materials, and for the sterilization of biologically-contaminated articles. The sterilization apparatus consists of layers of the resistive-barrier discharge device operating at room temperature, a sterilization chamber, and an ozone destruction device. An electrical discharge in the resistive-barrier discharge system generates an atmospheric plasma in oxygen gas, generating ozone, which in turn efficiently sterilizes medical tools and biologically contaminated articles at room temperature. A sterilization experiment was carried out at an apparatus volume of 100 liters, with a sterilization chamber volume of 60 liters, and a discharge device volume of 40 liters. The sterilization in this experiment required 60 W of power for 5 hours of residence time. For a given sterilization time, the required electrical power was proportional to the apparatus volume. Ozone in the sterilization chamber was destroyed safely after sterilization.

Numerical and experimental study on the dynamics of a μs helium plasma gun with various amounts of O2 admixture

NASA Astrophysics Data System (ADS)

Viegas, Pedro; Damany, Xavier; Iseni, Sylvain; Pouvesle, Jean-Michel; Robert, Eric; Bourdon, Anne

2016-09-01

The use of admixtures (mostly O2 and N2) to a helium buffer has been studied recently to tailor the generation of reactive species in plasma jets for biomedical applications. So far, most experiments have been dedicated to the study of the plasma plume. For endoscopic treatments, it is also important to better understand and optimize the propagation of discharges in long dielectric tubes as catheters. In this work, we present an experimental and numerical study on the dynamics of a μs helium plasma discharge with O2 admixture in a long dielectric tube. In simulations, a 2D fluid model is used. For comparison purposes, the geometries of the set-ups used for simulations and experiments are as close as possible. We compare experiments and simulations for different amounts of O2 admixture added to the buffer gas and present results on the velocity of the discharge front for the various amounts of O2 and different applied voltages. In order to study the influence of different amounts of O2 admixture on the helium discharge dynamics, detailed kinetic schemes have been used. The influence of Penning and charge exchange reactions on the discharge structure and dynamics are studied, as well as the role of negative ions. P.V. is supported by an EDOM fellowship, and X.D. by an INEL/Region Centre-Val de Loire fellowship.

Plasma Source Development for LAPD

NASA Astrophysics Data System (ADS)

Pribyl, P.; Gekelman, W.; Drandell, M.; Grunspen, S.; Nakamoto, M.; McBarron, A.

2003-10-01

The Large Plasma Device (LAPD) relies on an indirectly heated Barium Oxide (BaO) cathode to generate an extremely repeatable low-noise plasma. However there are two defects of this system: one is that the cathode is subject to oxygen poisoning in the event of accidental air leaks, requiring a lengthy recoating and regeneration process. Second, the indirect radiative heating is only about 50 % efficient, leading to a series of reliability issues. Alternate plasma sources are being investigated, including two types of directly heated BaO cathode and several configurations of inductively coupled RF plasmas. Direct heating for a cathode can be achieved either by embedding heaters within the nickel substrate, or by using inductive heating techniques to drive currents within the nickel itself. In both cases, the BaO coating still serves to emit the electrons and thus generate the plasma arc. An improved system would generate the plasma without the use of a "cathode" e.g. by inductively coupling energy directly into the plasma discharge. This technique is being investigated from the point of view of whether a) the bulk of the plasma column can be made sufficiently low-noise to be of experimental value and b) sufficiently dense plasmas can be formed.

Saddle antenna radio frequency ion sources

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dudnikov, V., E-mail: vadim@muonsinc.com; Johnson, R.; Murray, S.

Existing RF ion sources for accelerators have specific efficiencies for H{sup +} and H{sup −} ion generation ∼3–5 mA/cm{sup 2} kW, where about 50 kW of RF power is typically needed for 50 mA beam current production. The Saddle Antenna (SA) surface plasma source (SPS) described here was developed to improve H{sup −} ion production efficiency, reliability, and availability. In SA RF ion source, the efficiency of positive ion generation in the plasma has been improved to 200 mA/cm{sup 2} kW. After cesiation, the current of negative ions to the collector was increased from 1 mA to 10 mA withmore » RF power ∼1.5 kW in the plasma (6 mm diameter emission aperture) and up to 30 mA with ∼4 kW RF. Continuous wave (CW) operation of the SA SPS has been tested on the test stand. The general design of the CW SA SPS is based on the pulsed version. Some modifications were made to improve the cooling and cesiation stability. CW operation with negative ion extraction was tested with RF power up to ∼1.2 kW in the plasma with production up to Ic = 7 mA. A stable long time generation of H{sup −} beam without degradation was demonstrated in RF discharge with AlN discharge chamber.« less

METHOD OF PRODUCING ENERGETIC PLASMA FOR NEUTRON PRODUCTION

DOEpatents

Bell, P.R.; Simon, A.; Mackin, R.J. Jr.

1961-01-24

A method is given for producing an energetic plasma for neutron production. An energetic plasma is produced in a small magnetically confined subvolume of the device by providing a selected current of energetic molecular ions at least greater than that required for producing a current of atomic ions sufficient to achieve "burnout" of neutral particles in the subvolume. The atomic ions are provided by dissociation of the molecular ions by an energetic arc discharge within the subvolume. After burnout, the arc discharge is terminated, the magnetic fields increased, and cold fuel feed is substituted for the molecular ions. After the subvolume is filled with an energetic plasma, the size of the magnetically confined subvolume is gradually increased until the entire device is filled with an energetic neutron producing plasma. The reactions which take place in the device to produce neutrons will generate a certain amount of heat energy which may be converted by the use of a conventional heat cycle to produce electrical energy.

On the structure of pulsed plasma jets

NASA Astrophysics Data System (ADS)

Cavolowsky, John Arthur

A pulsed plasma jet is a turbulent, inhomogeneous fluid mechanical discharge capable of initiating and inhancing combustion. Having shown the ability to ignite lean fuel mixtures, is now offers the potential for real-time control of combustion processes. The fluid mechanical and chemical properties of such jets are explored. The fluid mechanical structure of the jet was examined using two optical diagnostic techniques. Self-light streak photography provided information on the motion of luminous gas particles in its core. The turbulent, thermal evolution of the jet was explored using high speed laser schlieren cinematography. By examine plasma jet generators with both opaque and transparent plasma cavities, detailed information on plasma formation and jet structure, beginning with the electric arc discharge in the cavity, was obtained. Molecular beam mass spectroscopy was used to determine temperature and species concentration in the jet. Both noncombustible and combustible jets were studied. Species measurements in combustible jets revealed significant concentrations of radicals and products of complete as well as incomplete combustion.

FAST TRACK COMMUNICATION: Plasma agents in bio-decontamination by dc discharges in atmospheric air

NASA Astrophysics Data System (ADS)

Machala, Zdenko; Chládeková, Lenka; Pelach, Michal

2010-06-01

Bio-decontamination of water and surfaces contaminated by bacteria (Salmonella typhimurium) was investigated in two types of positive dc discharges in atmospheric pressure air, in needle-to-plane geometry: the streamer corona and its transition to a novel regime called transient spark with short high current pulses of limited energy. Both generate a cold non-equilibrium plasma. Electro-spraying of treated water through a needle electrode was applied for the first time and resulted in fast bio-decontamination. Experiments providing separation of various biocidal plasma agents, along with the emission spectra and coupled with oxidation stress measurements in the cell membranes helped to better understand the mechanisms of microbial inactivation. The indirect exposure of contaminated surfaces to neutral active species was almost as efficient as the direct exposure to the plasma, whereas applying only UV radiation from the plasma had no biocidal effects. Radicals and reactive oxygen species were identified as dominant biocidal agents.

Analysis and experimental study on formation conditions of large-scale barrier-free diffuse atmospheric pressure air plasmas in repetitive pulse mode

NASA Astrophysics Data System (ADS)

Li, Lee; Liu, Lun; Liu, Yun-Long; Bin, Yu; Ge, Ya-Feng; Lin, Fo-Chang

2014-01-01

Atmospheric air diffuse plasmas have enormous application potential in various fields of science and technology. Without dielectric barrier, generating large-scale air diffuse plasmas is always a challenging issue. This paper discusses and analyses the formation mechanism of cold homogenous plasma. It is proposed that generating stable diffuse atmospheric plasmas in open air should meet the three conditions: high transient power with low average power, excitation in low average E-field with locally high E-field region, and multiple overlapping electron avalanches. Accordingly, an experimental configuration of generating large-scale barrier-free diffuse air plasmas is designed. Based on runaway electron theory, a low duty-ratio, high voltage repetitive nanosecond pulse generator is chosen as a discharge excitation source. Using the wire-electrodes with small curvature radius, the gaps with highly non-uniform E-field are structured. Experimental results show that the volume-scaleable, barrier-free, homogeneous air non-thermal plasmas have been obtained between the gap spacing with the copper-wire electrodes. The area of air cold plasmas has been up to hundreds of square centimeters. The proposed formation conditions of large-scale barrier-free diffuse air plasmas are proved to be reasonable and feasible.

Plasma-Based Mixing Actuation in Airflow, Quantitated by Probe Breakdown Fluorescence

NASA Astrophysics Data System (ADS)

Leonov, Sergey; Firsov, Alexander; Shurupov, Michail; Yarantsev, Dmitry; Ohio State University Team; JIHT RAS Team

2013-09-01

Effective mixing of fuel and oxidizer in air-breathing engine at compressible conditions is an essential problem of high-speed combustion due to short residence time of gas mixture in the combustor of limited length. The effect of the mixing actuation by plasma is observed because of the gasdynamic instability arisen after the long filamentary discharge of submicrosecond duration generated along the contact zone of two co-flown gases. The work is focused on detail consideration of the mechanism of gas instability, promoted by plasma, on effect of the discharge specific localization, and on diagnostics development for qualitative and quantitative estimation of the mixing efficiency. The dynamics of relative concentration of gas components is examined quantitatively by means of Probe Discharge Breakdown Fluorescence (PBF). In this method an optical emission spectra of weak filamentary high-voltage nanosecond probe discharge are collected from local zone of interest in airflow. The first measurements of the mixing efficiency in vicinity of wall-injected secondary gas are presented. It is shown that the method of PBF could deliver experimental data on state of the two-component medium with <1 mcs and <5 mm of time and spatial resolution, correspondingly. Funded by AFOSR under Dr Chiping Li supervision

Volumetric Near-Field Microwave Plasma Generation

NASA Technical Reports Server (NTRS)

Exton, R. J.; Balla, R. Jeffrey; Herring, G. C.; Popovic, S.; Vuskovic, L.

2003-01-01

A periodic series of microwave-induced plasmoids is generated using the outgoing wave from a microwave horn and the reflected wave from a nearby on-axis concave reflector. The plasmoids are spaced at half-wavelength separations according to a standing-wave pattern. The plasmoids are enhanced by an effective focusing in the near field of the horn (Fresnel region) as a result of a diffractive narrowing. Optical imaging, electron density, and rotational temperature measurements characterize the near field plasma region. Volumetric microwave discharges may have application to combustion ignition in scramjet engines.

Transpiration cooled electrodes and insulators for MHD generators

DOEpatents

Hoover, Jr., Delmer Q.

1981-01-01

Systems for cooling the inner duct walls in a magnetohydrodynamic (MHD) generator. The inner face components, adjacent the plasma, are formed of a porous material known as a transpiration material. Selected cooling gases are transpired through the duct walls, including electrically insulating and electrode segments, and into the plasma. A wide variety of structural materials and coolant gases at selected temperatures and pressures can be utilized and the gases can be drawn from the generation system compressor, the surrounding environment, and combustion and seed treatment products otherwise discharged, among many other sources. The conduits conducting the cooling gas are electrically insulated through low pressure bushings and connectors so as to electrically isolate the generator duct from the ground.

Temporal response of a surface flashover on a velvet cathode in a relativistic diode

DOE PAGES

Coleman, J. E.; Moir, D. C.; Crawford, M. T.; ...

2015-03-11

Surface flashover of a carbon fiber velvet cathode generates a discharge from which electrons are relativistically accelerated to γ ranging from 4.9 to 8.8 through a 17.8 cm diode. This discharge is assumed to be a hydrocarbon mixture. Our objective is to quantify the dynamics over the ~100 ns pulse of the plasma discharge generated on the surface of the velvet cathode and across the anode-cathode (A-K) gap. We present a qualitative comparison of calculated and measured results, which includes time resolved measurements with a photomultiplier tube and charge-coupled device images. Additionally, initial visible spectroscopy measurements will also be presentedmore » confirming the ion species are dominated by hydrogen.« less

OH Production Enhancement in Bubbling Pulsed Discharges

NASA Astrophysics Data System (ADS)

Lungu, Cristian P.; Porosnicu, Corneliu; Jepu, Ionut; Chiru, Petrica; Zaroschi, Valentin; Lungu, Ana M.; Saito, Nagahiro; Bratescu, Maria; Takai, Osamu; Velea, Theodor; Predica, Vasile

2010-10-01

The generation of active species, such as H2O2, O*, OH*, HO2*, O3, N2*, etc, produced in aqueous solutions by HV pulsed discharges was studied in order to find the most efficient way in waste water treatment taking into account that these species are almost stronger oxidizers than ozone. Plasma was generated inside gas bubbles formed by the argon, air and oxygen gas flow between the special designed electrodes. The pulse width and pulse frequency influence was studied in order to increase the efficiency of the OH active species formation. The produced active species were investigated by optical emission spectroscopy and correlated with electrical parameters of the discharges (frequency, pulse width, amplitude, and rise and decay time).

Surface plasma source with saddle antenna radio frequency plasma generator.

PubMed

Dudnikov, V; Johnson, R P; Murray, S; Pennisi, T; Piller, C; Santana, M; Stockli, M; Welton, R

2012-02-01

A prototype RF H(-) surface plasma source (SPS) with saddle (SA) RF antenna is developed which will provide better power efficiency for high pulsed and average current, higher brightness with longer lifetime and higher reliability. Several versions of new plasma generators with small AlN discharge chambers and different antennas and magnetic field configurations were tested in the plasma source test stand. A prototype SA SPS was installed in the Spallation Neutron Source (SNS) ion source test stand with a larger, normal-sized SNS AlN chamber that achieved unanalyzed peak currents of up to 67 mA with an apparent efficiency up to 1.6 mA∕kW. Control experiments with H(-) beam produced by SNS SPS with internal and external antennas were conducted. A new version of the RF triggering plasma gun has been designed. A saddle antenna SPS with water cooling is fabricated for high duty factor testing.

Influence of the RF electrode cleanliness on plasma characteristics and dust-particle generation in methane dusty plasmas

NASA Astrophysics Data System (ADS)

Géraud-Grenier, I.; Desdions, W.; Faubert, F.; Mikikian, M.; Massereau-Guilbaud, V.

2018-01-01

The methane decomposition in a planar RF discharge (13.56 MHz) leads both to a dust-particle generation in the plasma bulk and to a coating growth on the electrodes. Growing dust-particles fall onto the grounded electrode when they are too heavy. Thus, at the end of the experiment, the grounded electrode is covered by a coating and by fallen dust-particles. During the dust-particle growth, the negative DC self-bias voltage (VDC) increases because fewer electrons reach the RF electrode, leading to a more resistive plasma and to changes in the plasma chemical composition. In this paper, the cleanliness influence of the RF electrode on the dust-particle growth, on the plasma characteristics and composition is investigated. A cleanliness electrode is an electrode without coating and dust-particles on its surface at the beginning of the experiment.

Evolution of streamer groups in nonthermal plasma

NASA Astrophysics Data System (ADS)

Okubo, M.

2015-12-01

Nonthermal plasmas (NTPs) induced by atmospheric nanosecond pulsed corona discharge have been studied for controlling pollution from combustors, such as boilers, incinerators, and diesel engines. In high-speed short-width high-voltage pulsed corona discharge-induced plasmas, primary streamer evolution is followed by secondary streamer evolution. Though this phenomenon is known experimentally, the details of the structures of the streamers and their evolution mechanisms have not been fully clarified. In this letter, we perform quasi two-dimensional numerical analysis of nonequilibrium NTP induced by a nanosecond positive pulsed corona discharge. The continuum fluid equations for two-temperature nonequilibrium NTP are used as governing equations. In this study, 197 gas phase reactions for 25 chemical species and 21 surface reactions on the inner glass wall surface are considered in an air plasma under atmospheric pressure. The simulated behavior of the streamer groups agrees with experimental observations. Soon after the voltage increases on the reactor, primary streamers are formed, which may transit the complete gap, disappearing near the peak voltage. Next, second streamers appear, disappearing at the end of the applied voltage pulse. The streamer wavelength and the distance between the streamers in the axial direction are determined. Moreover, ozone generation is shown to be more significant in the secondary streamer. This simulation will allow better predictions for nanosecond positive pulsed plasma systems.

Potential of electric discharge plasma methods in abatement of volatile organic compounds originating from the food industry.

PubMed

Preis, S; Klauson, D; Gregor, A

2013-01-15

Increased volatile organic compounds emissions and commensurate tightening of applicable legislation mean that the development and application of effective, cost-efficient abatement methods are areas of growing concern. This paper reviews the last two decades' publications on organic vapour emissions from food processing, their sources, impacts and treatment methods. An overview of the latest developments in conventional air treatment methods is presented, followed by the main focus of the paper, non-thermal plasma technology. The results of the review suggest that non-thermal plasma technology, in its pulsed corona discharge configuration, is an emerging treatment method with potential for low-cost, effective abatement of a wide spectrum of organic air pollutants. It is found that the combination of plasma treatment with catalysis is a development trend that demonstrates considerable potential. The as yet relatively small number of plasma treatment applications is considered to be due to the novelty of pulsed electric discharge techniques and a lack of reliable pulse generators and reactors. Other issues acting as barriers to widespread adoption of the technique include the possible formation of stable oxidation by-products, residual ozone and nitrogen oxides, and sensitivity towards air humidity. Copyright © 2012 Elsevier Ltd. All rights reserved.

Nanosecond Surface Microdischarges in Multilayer Structures

NASA Astrophysics Data System (ADS)

Dubinov, A. E.; Lyubimtseva, V. A.

2018-05-01

Multilayer structures in which nanosecond surface microdischarges are generated have been developed, fabricated, and investigated. In these structures, layers are made in the form of thin transparent films, and a plasma discharge channel is formed in thin spacings between the layers. Passage of the discharge channel from one layer into the neighboring layer is implemented via pre-fabricated microholes. Images of microdischarges were obtained which confirmed that their plasma channels are formed according to the route assigned by the holes. The route may follow a fairly complex scheme and have self-intersection points and portions in which the electrons are bound to move in opposition to the electric field. In studying the shape of channels in multilayer strictures, the authors have found a new physical effect which lies in the azimuthal self-orientation of the discharge channel as it passes from one microhole to another.

2D laser-collision induced fluorescence in low-pressure argon discharges

DOE PAGES

Barnat, E. V.; Weatherford, B. R.

2015-09-25

Development and application of laser-collision induced fluorescence (LCIF) diagnostic technique is presented for the use of interrogating argon plasma discharges. Key atomic states of argon utilized for the LCIF method are identified. A simplified two-state collisional radiative model is then used to establish scaling relations between the LCIF, electron density, and reduced electric fields ( E/N). The procedure used to generate, detect and calibrate the LCIF in controlled plasma environments is discussed in detail. LCIF emanating from an argon discharge is then presented for electron densities spanning 10 9 e cm –3 to 10 12 e cm –3 and reducedmore » electric fields spanning 0.1 Td to 40 Td. Lastly, application of the LCIF technique for measuring the spatial distribution of both electron densities and reduced electric field is demonstrated.« less

Experimental and computational study of dielectric barrier discharges for environmental applications

NASA Astrophysics Data System (ADS)

Aerts, Robby

Air pollution has become a major global concern which affects all inhabitants of our precious earth. Nowadays it is fact that our climate is changing and the sea level is rising. Moreover, we are facing an energy crisis because all our fossil fuel resources will sooner or later be running empty. It is clear that drastic measures are needed to keep our planet as it is today for generations to come. One of these measures is the 20-20-20 targets imposed by the European Commission, which stimulates the research for environmental energy applications. In this PhD dissertation two environmental applications of plasma technology are investigated. The first one is the abatement of flue gases, and more specifically the destruction of volatile organic compounds (VOCs). The second one is the conversion of CO2 into valuable chemicals. Both of these applications suffer from a large energy cost under classical (thermodynamic) conditions, due to the chemical stability of these molecules. Plasma technology is quite promising to overcome these thermodynamic barriers. Plasmas allow reactions at different time-scales with different species, such as electrons, ions, radicals, molecules and excited species, creating new chemical pathways. Indeed, in a plasma the applied electrical energy is directly transferred to the electrons, which activate the gas by ionization, excitation and dissociation, hence creating reactive species (ions, excited species, radicals), that can further easily undergo other chemical reactions. Especially gas discharges, which are low temperature plasmas, show promising results in the destruction of pollutants at mild conditions. A common type of gas discharge is the dielectric barrier discharge (DBD) which has been successfully scaled up for industrial ozone generation and is widely investigated in the field of environmental applications. The complexity of DBDs creates difficulties for experimental diagnostics and therefore numerical studies can help to improve our understanding of the ongoing processes. A chemical kinetics model developed by M. Kushner and co-workers combined with experiments was used in this PhD dissertation to obtain insight in the ongoing plasma chemistry for the environmental applications discussed above.

Direct and Efficient Dehydrogenation of Tetrahydroquinolines and Primary Amines Using Corona Discharge Generated on Ambient Hydrophobic Paper Substrate.

PubMed

Davis, Kathryn M; Badu-Tawiah, Abraham K

2017-04-01

The exposure of an aqueous-based liquid drop containing amines and graphite particles to plasma generated by a corona discharge results in heterogeneous aerobic dehydrogenation reactions. This green oxidation reaction occurring in ambient air afforded the corresponding quinolines and nitriles from tetrahydroquinolines and primary amines, respectively, at >96% yields in less than 2 min of reaction time. The accelerated dehydrogenation reactions occurred on the surface of a low energy hydrophobic paper, which served both as container for holding the reacting liquid drop and as a medium for achieving paper spray ionization of reaction products for subsequent characterization by ambient mass spectrometry. Control experiments indicate superoxide anions (O 2 •- ) are the main reactive species; the presence of graphite particles introduced heterogeneous surface effects, and enabled the efficient sampling of the plasma into the grounded analyte droplet solution. Graphical Abstract ᅟ.

Direct and Efficient Dehydrogenation of Tetrahydroquinolines and Primary Amines Using Corona Discharge Generated on Ambient Hydrophobic Paper Substrate

NASA Astrophysics Data System (ADS)

Davis, Kathryn M.; Badu-Tawiah, Abraham K.

2017-04-01

The exposure of an aqueous-based liquid drop containing amines and graphite particles to plasma generated by a corona discharge results in heterogeneous aerobic dehydrogenation reactions. This green oxidation reaction occurring in ambient air afforded the corresponding quinolines and nitriles from tetrahydroquinolines and primary amines, respectively, at >96% yields in less than 2 min of reaction time. The accelerated dehydrogenation reactions occurred on the surface of a low energy hydrophobic paper, which served both as container for holding the reacting liquid drop and as a medium for achieving paper spray ionization of reaction products for subsequent characterization by ambient mass spectrometry. Control experiments indicate superoxide anions (O2 •-) are the main reactive species; the presence of graphite particles introduced heterogeneous surface effects, and enabled the efficient sampling of the plasma into the grounded analyte droplet solution.

Analysis and design of ion thrusters for large space systems

NASA Technical Reports Server (NTRS)

James, E. L.

1980-01-01

This study undertakes the analysis and conceptual design of a 0.5 Newton electrostatic ion thruster suitable for use on large space system missions in the next decade. Either argon or xenon gas shall be used as propellant. A 50 cm diameter discharge chamber was selected to meet stipulated performance goals. The discharge plasma is contained at the boundary by a periodic structure of alternating permanent magnets generating a series of line cusps. Anode strips between the magnets collect Maxwellian electrons generated by a central cathode. Ion extraction utilizes either two or three grid optics at the user's choice. An extensive analysis was undertaken to investigate optics behavior in the high power environment of this large thruster. A plasma bridge neutralizer operating on inert gas provides charge neutralizing electrons to complete the design. The resulting conceptual thruster and the necessary power management and control requirements are described.

Contact Geometry and Distribution of Plasma Generated in the Vicinity of Sliding Contact

NASA Astrophysics Data System (ADS)

Nakayama, Keiji

2007-09-01

The effect of the geometry of the smaller sliding partner on plasma (triboplasma) generation has been investigated as a function of the tip radius of a diamond pin, which slides against a single crystal sapphire disk under atmospheric dry air pressure. It was found that the diameter and the total intensity of the circular triboplasma increase parabolically with an increase in the tip radius of the pin under constant normal force and sliding velocity. The plasma is most intense at the crossing point of the plasma ring and the frictional track in the plasma circle. The gap distance at the crossing point is independent of the tip radius. The ring diameter increases with an increase in the tip radius, keeping the gap distance constant and obeying Paschen’s law of gas discharge.

Diagnostics of hydrogen plasma with in situ optical emission and silicon probes

NASA Astrophysics Data System (ADS)

Lee, Szetsen; Chung, Yi-Jie

2005-11-01

In this work, an approach has been adopted to explore plasma properties by combining an in situ optical emission technique with a contact angle measurement. Hydrogen plasma was generated with a radio-frequency power source. The plasma parameters such as number densities and temperatures were derived from the optical emission spectroscopic data. Small silicon chips were placed at various positions inside a discharge tube as probes for the plasma conditions. The hydrogen-plasma-treated silicon chip surfaces were characterized with the contact angle measurement method. The change of wettability on the silicon surface was observed with various plasma treatment times. The spectroscopic information about the plasma is correlated with the results of the surface characterization. It is found that the rate of the increasing hydrophilicity is sensitive to the amount of helium added and the location in the discharge tube. A simple model describing the relation between the surface coverage area of water droplet and the variation of contact angle has been established. We have proposed plasma excitation and reaction mechanisms for the observed correlation between plasma temperatures and the wettability of the silicon surface. It shows that small silicon chips can serve as "litmus tests" for the plasma conditions without introducing too much perturbation.

Yield of H2O2 in Gas-Liquid Phase with Pulsed DBD

NASA Astrophysics Data System (ADS)

Jiang, Song; Wen, Yiyong; Liu, Kefu

2014-01-01

Electric discharge in water can generate a large number of oxidants such as ozone, hydrogen peroxide and hydroxyl radicals. In this paper, a non-thermal plasma processing system was established by means of pulsed dielectric barrier discharge in gas-liquid phase. The electrodes of discharge reactor were staggered. The yield of H2O2 was enhanced after discharge. The effects of discharge time, discharge voltage, frequency, initial pH value, and feed gas were investigated. The concentration of hydrogen peroxide and ozone was measured after discharge. The experimental results were fully analyzed. The chemical reaction equations in water were given as much as possible. At last, the water containing Rhodamine B was tested in this system. The degradation rate came to 94.22% in 30 min.

A power-balance model for local helicity injection startup in a spherical tokamak

DOE Office of Scientific and Technical Information (OSTI.GOV)

Barr, Jayson L.; Bongard, Michael W.; Burke, Marcus G.

A 0D circuit model for predicting I p( t) in Local Helicity Injection (LHI) discharges is developed. Analytic formulas for estimating the surface flux of finite-A plasmas developed are modified and expanded to treat highly shaped, ultralow-A tokamak geometry using a database of representative equilibria. Model predictions are compared to sample LHI discharges in the A ~ 1 Pegasus spherical tokamak, and are found to agree within 15% of experimental I p( t). High performance LHI discharges are found to follow the Taylor relaxation current limit for approximately the first half of the current ramp, or I p ≲ 75more » kA. The second half of the current ramp follows a limit imposed by power-balance as plasmas expand from high- A to ultralow- A. Here, this shape evolution generates a significant drop in external plasma inductance, effectively using the plasma’s initially high inductance to drive the current ramp and provide > 70% of the current drive V-s. Projections using this model indicate the relative influences of higher helicity input rate and injector current on the attainable total plasma current.« less

A power-balance model for local helicity injection startup in a spherical tokamak

DOE PAGES

Barr, Jayson L.; Bongard, Michael W.; Burke, Marcus G.; ...

2018-05-15

A 0D circuit model for predicting I p( t) in Local Helicity Injection (LHI) discharges is developed. Analytic formulas for estimating the surface flux of finite-A plasmas developed are modified and expanded to treat highly shaped, ultralow-A tokamak geometry using a database of representative equilibria. Model predictions are compared to sample LHI discharges in the A ~ 1 Pegasus spherical tokamak, and are found to agree within 15% of experimental I p( t). High performance LHI discharges are found to follow the Taylor relaxation current limit for approximately the first half of the current ramp, or I p ≲ 75more » kA. The second half of the current ramp follows a limit imposed by power-balance as plasmas expand from high- A to ultralow- A. Here, this shape evolution generates a significant drop in external plasma inductance, effectively using the plasma’s initially high inductance to drive the current ramp and provide > 70% of the current drive V-s. Projections using this model indicate the relative influences of higher helicity input rate and injector current on the attainable total plasma current.« less

Fundamental Studies of Electric-Field-Induced Coherent Raman Scattering

DTIC Science & Technology

2011-06-07

denote by IIR and ICARS , may be written [1,5] as   22121 EIINNCI exgIR  (1) and   22122 IINNCI exgCARS  , (2) where C1 and C2 are...biological applications [8-11], and aerodynamic controls [12]. A better understanding of the discharge mechanisms of such plasmas is expected to contribute to...the development of better plasma generation systems specific for each application. When APPs are used with low gas temperature, plasmas are

Study on Formation of Plasma Nanobubbles in Water

NASA Astrophysics Data System (ADS)

Sato, Takehiko; Nakatani, Tatsuyuki; Miyahara, Takashi; Ochiai, Shiroh; Oizumi, Masanobu; Fujita, Hidemasa; Miyazaki, Takamichi

2015-12-01

Nanobubbles of less than 400 nm in diameter were formed by plasma in pure water. Pre-breakdown plasma termed streamer discharges, generated gas channels shaped like fine dendritic coral leading to the formation of small bubbles. Nanobubbles were visualized by an optical microscope and measured by dynamic laser scattering. However, it is necessary to verify that these nanobubbles are gas bubbles, not solid, because contamination such as platinum particles and organic compounds from electrode and residue in ultrapure water were also observed.

Low pass filter for plasma discharge

DOEpatents

Miller, Paul A.

1994-01-01

An isolator is disposed between a plasma reactor and its electrical energy source in order to isolate the reactor from the electrical energy source. The isolator operates as a filter to attenuate the transmission of harmonics of a fundamental frequency of the electrical energy source generated by the reactor from interacting with the energy source. By preventing harmonic interaction with the energy source, plasma conditions can be readily reproduced independent of the electrical characteristics of the electrical energy source and/or its associated coupling network.

Multi-cathode metal vapor arc ion source

DOEpatents

Brown, Ian G.; MacGill, Robert A.

1988-01-01

An ion generating apparatus utilizing a vacuum chamber, a cathode and an anode in the chamber. A source of electrical power produces an arc or discharge between the cathode and anode. The arc is sufficient to vaporize a portion of the cathode to form a plasma. The plasma is directed to an extractor which separates the electrons from the plasma, and accelerates the ions to produce an ion beam. One embodiment of the appaatus utilizes a multi-cathode arrangement for interaction with the anode.

Particle based plasma simulation for an ion engine discharge chamber

NASA Astrophysics Data System (ADS)

Mahalingam, Sudhakar

Design of the next generation of ion engines can benefit from detailed computer simulations of the plasma in the discharge chamber. In this work a complete particle based approach has been taken to model the discharge chamber plasma. This is the first time that simplifying continuum assumptions on the particle motion have not been made in a discharge chamber model. Because of the long mean free paths of the particles in the discharge chamber continuum models are questionable. The PIC-MCC model developed in this work tracks following particles: neutrals, singly charged ions, doubly charged ions, secondary electrons, and primary electrons. The trajectories of these particles are determined using the Newton-Lorentz's equation of motion including the effects of magnetic and electric fields. Particle collisions are determined using an MCC statistical technique. A large number of collision processes and particle wall interactions are included in the model. The magnetic fields produced by the permanent magnets are determined using Maxwell's equations. The electric fields are determined using an approximate input electric field coupled with a dynamic determination of the electric fields caused by the charged particles. In this work inclusion of the dynamic electric field calculation is made possible by using an inflated plasma permittivity value in the Poisson solver. This allows dynamic electric field calculation with minimal computational requirements in terms of both computer memory and run time. In addition, a number of other numerical procedures such as parallel processing have been implemented to shorten the computational time. The primary results are those modeling the discharge chamber of NASA's NSTAR ion engine at its full operating power. Convergence of numerical results such as total number of particles inside the discharge chamber, average energy of the plasma particles, discharge current, beam current and beam efficiency are obtained. Steady state results for the particle number density distributions and particle loss rates to the walls are presented. Comparisons of numerical results with experimental measurements such as currents and the particle number density distributions are made. Results from a parametric study and from an alternative magnetic field design are also given.

Growth and male reproduction improvement of non-thermal dielectric barrier discharge plasma treatment on chickens

NASA Astrophysics Data System (ADS)

Jiao Zhang, Jiao; Luong Huynh, Do; Chandimali, Nisansala; Kang, Tae Yoon; Kim, Nameun; Mok, Young Sun; Kwon, Taeho; Jeong, Dong Kee

2018-05-01

This study investigated whether plasma treatment of fertilized eggs before hatching could affect the growth and reproduction of chickens. Three point five-day-incubated fertilized eggs exposed to non-thermal dielectric barrier discharge plasma at 2.81 W of power for 2 min resulted in the highest growth in chickens. Plasma growth-promoting effect was regulated by the reactive oxygen species homeostasis and the improvement of energy metabolism via increasing serum hormones and adenosine triphosphate levels which were resulted from the regulation of genes involved in antioxidant defense, hormone biosynthesis and energetic metabolism. Interestingly, plasma-treated male chickens conspicuously grew faster than females. Further, aspects of male reproductive system (testosterone level and sperm quality) were improved by the plasma treatment but female reproduction (estradiol and progesterone levels, egg-laying rate and egg weight) had no significant changes. Unfortunately, offspring whose parents were the optimal plasma-treated chickens did not show any difference on growth characteristics and failed to inherit excellent growth features from their parents. Our results suggest a new method to improve the growth rate and male reproductive capacity in poultry but it is only effective in the plasma direct-treated generation.

Fast plasma shutdown by killer pellet injection in JT-60U with reduced heat flux on the divertor plate and avoiding runaway electron generation

NASA Astrophysics Data System (ADS)

Yoshino, R.; Kondoh, T.; Neyatani, Y.; Itami, K.; Kawano, Y.; Isei, N.

1997-02-01

A killer pellet is an impurity pellet that is injected into a tokamak plasma in order to terminate a discharge without causing serious damage to the tokamak machine. In JT-60U neon ice pellets have been injected into OH and NB heated plasmas and fast plasma shutdowns have been demonstrated without large vertical displacement. The heat pulse on the divertor plate has been greatly reduced by killer pellet injection (KPI), but a low-power heat flux tail with a long time duration is observed. The total energy on the divertor plate increases with longer heat flux tail, so it has been reduced by shortening the tail. Runaway electron (RE) generation has been observed just after KPI and/or in the later phase of the plasma current quench. However, RE generation has been avoided when large magnetic perturbations are excited. These experimental results clearly show that KPI is a credible fast shutdown method avoiding large vertical displacement, reducing heat flux on the divertor plate, and avoiding (or minimizing) RE generation.

Nonthermal dielectric-barrier discharge plasma-induced inactivation involves oxidative DNA damage and membrane lipid peroxidation in Escherichia coli.

PubMed

Joshi, Suresh G; Cooper, Moogega; Yost, Adam; Paff, Michelle; Ercan, Utku K; Fridman, Gregory; Friedman, Gary; Fridman, Alexander; Brooks, Ari D

2011-03-01

Oxidative stress leads to membrane lipid peroxidation, which yields products causing variable degrees of detrimental oxidative modifications in cells. Reactive oxygen species (ROS) are the key regulators in this process and induce lipid peroxidation in Escherichia coli. Application of nonthermal (cold) plasma is increasingly used for inactivation of surface contaminants. Recently, we reported a successful application of nonthermal plasma, using a floating-electrode dielectric-barrier discharge (FE-DBD) technique for rapid inactivation of bacterial contaminants in normal atmospheric air (S. G. Joshi et al., Am. J. Infect. Control 38:293-301, 2010). In the present report, we demonstrate that FE-DBD plasma-mediated inactivation involves membrane lipid peroxidation in E. coli. Dose-dependent ROS, such as singlet oxygen and hydrogen peroxide-like species generated during plasma-induced oxidative stress, were responsible for membrane lipid peroxidation, and ROS scavengers, such as α-tocopherol (vitamin E), were able to significantly inhibit the extent of lipid peroxidation and oxidative DNA damage. These findings indicate that this is a major mechanism involved in FE-DBD plasma-mediated inactivation of bacteria.

Nonthermal Dielectric-Barrier Discharge Plasma-Induced Inactivation Involves Oxidative DNA Damage and Membrane Lipid Peroxidation in Escherichia coli▿

PubMed Central

Joshi, Suresh G.; Cooper, Moogega; Yost, Adam; Paff, Michelle; Ercan, Utku K.; Fridman, Gregory; Friedman, Gary; Fridman, Alexander; Brooks, Ari D.

2011-01-01

Oxidative stress leads to membrane lipid peroxidation, which yields products causing variable degrees of detrimental oxidative modifications in cells. Reactive oxygen species (ROS) are the key regulators in this process and induce lipid peroxidation in Escherichia coli. Application of nonthermal (cold) plasma is increasingly used for inactivation of surface contaminants. Recently, we reported a successful application of nonthermal plasma, using a floating-electrode dielectric-barrier discharge (FE-DBD) technique for rapid inactivation of bacterial contaminants in normal atmospheric air (S. G. Joshi et al., Am. J. Infect. Control 38:293-301, 2010). In the present report, we demonstrate that FE-DBD plasma-mediated inactivation involves membrane lipid peroxidation in E. coli. Dose-dependent ROS, such as singlet oxygen and hydrogen peroxide-like species generated during plasma-induced oxidative stress, were responsible for membrane lipid peroxidation, and ROS scavengers, such as α-tocopherol (vitamin E), were able to significantly inhibit the extent of lipid peroxidation and oxidative DNA damage. These findings indicate that this is a major mechanism involved in FE-DBD plasma-mediated inactivation of bacteria. PMID:21199923

Large area multiarc ion beam source {open_quote}MAIS{close_quote}

DOE Office of Scientific and Technical Information (OSTI.GOV)

Engelko, V.; Giese, H.; Schalk, S.

1996-12-31

A pulsed large area intense ion beam source is described, in which the ion emitting plasma is built up by an array of individual discharge units, homogeneously distributed over the surface of a common discharge electrode. A particularly advantageous feature of the source is that for plasma generation and subsequent acceleration of the ions only one common energy supply is necessary. This allows to simplify the source design and provides inherent synchronization of plasma production and ion extraction. The homogeneity of the plasma density was found to be superior to plasma sources using plasma expanders. Originally conceived for the productionmore » of proton beams, the source can easily be modified for the production of beams composed of carbon and metal ions or mixed ion species. Results of investigations of the source performance for the production of a proton beam are presented. The maximum beam current achieved to date is of the order of 100 A, with a particle kinetic energy of 15 - 30 keV and a pulse length in the range of 10 {mu}s.« less

Signal enhancement in laser-induced breakdown spectroscopy using fast square-pulse discharges

NASA Astrophysics Data System (ADS)

Sobral, H.; Robledo-Martinez, A.

2016-10-01

A fast, high voltage square-shaped electrical pulse initiated by laser ablation was investigated as a means to enhance the analytical capabilities of laser Induced breakdown spectroscopy (LIBS). The electrical pulse is generated by the discharge of a charged coaxial cable into a matching impedance. The pulse duration and the stored charge are determined by the length of the cable. The ablation plasma was produced by hitting an aluminum target with a nanosecond 532-nm Nd:YAG laser beam under variable fluence 1.8-900 J cm- 2. An enhancement of up to one order of magnitude on the emission signal-to-noise ratio can be achieved with the spark discharge assisted laser ablation. Besides, this increment is larger for ionized species than for neutrals. LIBS signal is also increased with the discharge voltage with a tendency to saturate for high laser fluences. Electron density and temperature evolutions were determined from time delays of 100 ns after laser ablation plasma onset. Results suggest that the spark discharge mainly re-excites the laser produced plume.

Experimental demonstration of plasma startup by coaxial helicity injection

NASA Astrophysics Data System (ADS)

Raman, R.; Jarboe, T. R.; Nelson, B. A.; Hamp, W. T.; Izzo, V. A.; O'Neill, R. G.; Redd, A. J.; Sieck, P. E.; Smith, R. J.

2004-05-01

Experimental results on the transfer of a coaxial-helicity-injection (CHI) produced discharge to inductive operation are reported. CHI assisted plasma startup is more robust than inductive only operation and reduces volt-seconds consumption. After handoff to inductive operation, the initial 100 kA of CHI produced current drops to 50 kA, then ramps up to 180 kA, using only 30 mVs, about 40% higher than that produced by induction alone. Results show that initiation of CHI discharges at lower densities produce higher levels of coupling current. Coupling a CHI produced discharge to induction from a precharged central solenoid has produced record currents of 290 kA using only 52 mWb of central solenoid flux. CHI discharges can also be generated while the central transformer is in the process of being precharged, during which period it induces a negative loop voltage on the CHI discharge. These significant results were obtained on the Helicity Injected Torus-II (HIT-II) [T.R. Jarboe, Fusion Technol. 15, 7 (1989)] spherical torus experiment (major/minor radius of 0.3/0.2 m and elongation of 1.5).

Pulsed-Plasma Disinfection of Water Containing Escherichia coli

NASA Astrophysics Data System (ADS)

Satoh, Kohki; MacGregor, Scott J.; Anderson, John G.; Woolsey, Gerry A.; Fouracre, R. Anthony

2007-03-01

The disinfection of water containing the microorganism, Escherichia coli (E. coli) by exposure to a pulsed-discharge plasma generated above the water using a multineedle electrode (plasma-exposure treatment), and by sparging the off-gas of the pulsed plasma into the water (off-gas-sparging treatment), is performed in the ambient gases of air, oxygen, and nitrogen. For the off-gas-sparging treatment, bactericidal action is observed only when oxygen is used as the ambient gas, and ozone is found to generate the bactericidal action. For the plasma-exposure treatment, the density of E. coli bacteria decreases exponentially with plasma-exposure time for all the ambient gases. It may be concluded that the main contributors to E. coli inactivation are particle species produced by the pulsed plasma. For the ambient gases of air and nitrogen, the influence of acidification of the water in the system, as a result of pulsed-plasma exposure, may also contribute to the decay of E. coli density.

Electron density in surface barrier discharge emerging at argon/water interface: quantification for streamers and leaders

NASA Astrophysics Data System (ADS)

Cvetanović, Nikola; Galmiz, Oleksandr; Synek, Petr; Zemánek, Miroslav; Brablec, Antonín; Hoder, Tomáš

2018-02-01

Optical emission spectroscopy, fast intensified CCD imaging and electrical measurements were applied to investigate the basic plasma parameters of surface barrier discharge emerging from a conductive water electrode. The discharge was generated at the triple-line interface of atmospheric pressure argon gas and conductive water solution at the fused silica dielectrics using a sinusoidal high-voltage waveform. The spectroscopic methods of atomic line broadening and molecular spectroscopy were used to determine the electron densities and the gas temperature in the active plasma. These parameters were obtained for both applied voltage polarities and resolved spatially. Two different spectral signatures were identified in the spatially resolved spectra resulting in electron densities differing by two orders of magnitude. It is shown that two discharge mechanisms take a place: the streamer and the leader one, with electron densities of 1014 and 1016 cm-3, respectively. This spectroscopic evidence is supported by the combined diagnostics of electrical current measurements and phase-resolved intensified CCD camera imaging.

Energy & mass-charge distribution peculiarities of ion emitted from penning source

NASA Astrophysics Data System (ADS)

Mamedov, N. V.; Kolodko, D. V.; Sorokin, I. A.; Kanshin, I. A.; Sinelnikov, D. N.

2017-05-01

The optimization of hydrogen Penning sources used, in particular, in plasma chemical processing of materials and DLC deposition, is still very important. Investigations of mass-charge composition of these ion source emitted beams are particular relevant for miniature linear accelerators (neutron flux generators) nowadays. The Penning ion source energy and mass-charge ion distributions are presented. The relation between the discharge current abrupt jumps with increasing plasma density in the discharge center and increasing potential whipping (up to 50% of the anode voltage) is shown. Also the energy spectra in the discharge different modes as the pressure and anode potential functions are presented. It has been revealed that the atomic hydrogen ion concentration is about 5-10%, and it weakly depends on the pressure and the discharge current (in the investigated range from 1 to 10 mTorr and from 50 to 1000 μA) and increases with the anode voltage (up 1 to 3,5 kV).

Bioactive surface modifications on inner walls of poly-tetra-fluoro-ethylene tubes using dielectric barrier discharge

NASA Astrophysics Data System (ADS)

Cho, Yong Ki; Park, Daewon; Kim, Hoonbae; Lee, Hyerim; Park, Heonyong; Kim, Hong Ja; Jung, Donggeun

2014-03-01

Bioactive surface modification can be used in a variety of medical polymeric materials in the fields of biochips and biosensors, artificial membranes, and vascular grafts. In this study, the surface modification of the inner walls of poly-tetra-fluoro-ethylene (PTFE) tubing was carried out to improve vascular grafts, which are made of biocompatible material for the human body in the medical field. Focus was centered on the cell attachment of the inner wall of the PTFE by sequential processes of hydrogen plasma treatment, hydrocarbon deposition, and reactive plasma treatment on the PFTE surface using micro plasma discharge. Micro plasma was generated by a medium-frequency alternating current high-voltage generator. The preliminary modification of PTFE was conducted by a plasma of hydrogen and argon gases. The hydrocarbon thin film was deposited on modified PTFE with a mixture of acetylene and argon gases. The reactive plasma treatment using oxygen plasma was done to give biocompatible functionality to the inner wall surface. The hydrophobic surface of bare PTFE is made hydrophilic by the reactive plasma treatment due to the formation of carbonyl groups on the surface. The reactive treatment could lead to improved attachment of smooth muscle cells (SMCs) on the modified PTFE tubing. Fourier transform infrared absorption spectroscopy, X-ray photoelectron spectroscopy, scanning electron microscopy, and water contact angle measurement were used for the analysis of the surface modification. The SMC-attached PTFE tube developed will be applicable to in vitro human vasculature-mimetic model systems, and to medical vascular grafts.

PLASMA GENERATOR

DOEpatents

Wilcox, J.M.; Baker, W.R.

1963-09-17

This invention is a magnetohydrodynamic device for generating a highly ionized ion-electron plasma at a region remote from electrodes and structural members, thus avoiding contamination of the plasma. The apparatus utilizes a closed, gas-filled, cylindrical housing in which an axially directed magnetic field is provided. At one end of the housing, a short cylindrical electrode is disposed coaxially around a short axial inner electrode. A radial electrical discharge is caused to occur between the inner and outer electrodes, creating a rotating hydromagnetic ionization wave that propagates aiong the magnetic field lines toward the opposite end of the housing. A shorting switch connected between the electrodes prevents the wave from striking the opposite end of the housing. (AEC)

Connection between plasma response and resonant magnetic perturbation (RMP) edge localized mode (ELM) suppression in DIII-D [Connection between plasma response and RMP ELM suppression in DIII-D

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wingen, Andreas; Ferraro, Nathaniel M.; Shafer, Morgan W.

Calculations of the plasma response to applied non-axisymmetric fields in several DIII-D discharges show that predicted displacements depend strongly on the edge current density. This result is found using both a linear two-fluid-MHD model (M3D-C1) and a nonlinear ideal-MHD model (VMEC). Furthermore, it is observed that the probability of a discharge being edge localized mode (ELM)-suppressed is most closely related to the edge current density, as opposed to the pressure gradient. It is found that discharges with a stronger kink response are closer to the peeling–ballooning stability limit in ELITE simulations and eventually cross into the unstable region, causing ELMsmore » to reappear. Thus for effective ELM suppression, the RMP has to prevent the plasma from generating a large kink response, associated with ELM instability. Experimental observations are in agreement with the finding; discharges which have a strong kink response in the MHD simulations show ELMs or ELM mitigation during the RMP phase of the experiment, while discharges with a small kink response in the MHD simulations are fully ELM suppressed in the experiment by the applied resonant magnetic perturbation. The results are cross-checked against modeled 3D ideal MHD equilibria using the VMEC code. The procedure of constructing optimal 3D equilibria for diverted H-mode discharges using VMEC is presented. As a result, kink displacements in VMEC are found to scale with the edge current density, similar to M3D-C1, but the displacements are smaller. A direct correlation in the flux surface displacements to the bootstrap current is shown.« less

Connection between plasma response and resonant magnetic perturbation (RMP) edge localized mode (ELM) suppression in DIII-D [Connection between plasma response and RMP ELM suppression in DIII-D

DOE PAGES

Wingen, Andreas; Ferraro, Nathaniel M.; Shafer, Morgan W.; ...

2015-09-03

Calculations of the plasma response to applied non-axisymmetric fields in several DIII-D discharges show that predicted displacements depend strongly on the edge current density. This result is found using both a linear two-fluid-MHD model (M3D-C1) and a nonlinear ideal-MHD model (VMEC). Furthermore, it is observed that the probability of a discharge being edge localized mode (ELM)-suppressed is most closely related to the edge current density, as opposed to the pressure gradient. It is found that discharges with a stronger kink response are closer to the peeling–ballooning stability limit in ELITE simulations and eventually cross into the unstable region, causing ELMsmore » to reappear. Thus for effective ELM suppression, the RMP has to prevent the plasma from generating a large kink response, associated with ELM instability. Experimental observations are in agreement with the finding; discharges which have a strong kink response in the MHD simulations show ELMs or ELM mitigation during the RMP phase of the experiment, while discharges with a small kink response in the MHD simulations are fully ELM suppressed in the experiment by the applied resonant magnetic perturbation. The results are cross-checked against modeled 3D ideal MHD equilibria using the VMEC code. The procedure of constructing optimal 3D equilibria for diverted H-mode discharges using VMEC is presented. As a result, kink displacements in VMEC are found to scale with the edge current density, similar to M3D-C1, but the displacements are smaller. A direct correlation in the flux surface displacements to the bootstrap current is shown.« less

Runaway electron generation as possible trigger for enhancement of magnetohydrodynamic plasma activity and fast changes in runaway beam behavior

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pankratov, I. M., E-mail: pankratov@kipt.kharkov.ua, E-mail: rjzhou@ipp.ac.cn; Zhou, R. J., E-mail: pankratov@kipt.kharkov.ua, E-mail: rjzhou@ipp.ac.cn; Hu, L. Q.

2015-07-15

Peculiar phenomena were observed during experiments with runaway electrons: rapid changes in the synchrotron spot and its intensity that coincided with stepwise increases in the electron cyclotron emission (ECE) signal (cyclotron radiation of suprathermal electrons). These phenomena were initially observed in TEXTOR (Tokamak Experiment for Technology Oriented Research), where these events only occurred in the current decay phase or in discharges with thin stable runaway beams at a q = 1 drift surface. These rapid changes in the synchrotron spot were interpreted by the TEXTOR team as a fast pitch angle scattering event. Recently, similar rapid changes in the synchrotron spot andmore » its intensity that coincided with stepwise increases in the non-thermal ECE signal were observed in the EAST (Experimental Advanced Superconducting Tokamak) runaway discharge. Runaway electrons were located around the q = 2 rational magnetic surface (ring-like runaway electron beam). During the EAST runaway discharge, stepwise ECE signal increases coincided with enhanced magnetohydrodynamic (MHD) activity. This behavior was peculiar to this shot. In this paper, we show that these non-thermal ECE step-like jumps were related to the abrupt growth of suprathermal electrons induced by bursting electric fields at reconnection events during this MHD plasma activity. Enhancement of the secondary runaway electron generation also occurred simultaneously. Local changes in the current-density gradient appeared because of local enhancement of the runaway electron generation process. These current-density gradient changes are considered to be a possible trigger for enhancement of the MHD plasma activity and the rapid changes in runaway beam behavior.« less

Runaway electron generation as possible trigger for enhancement of magnetohydrodynamic plasma activity and fast changes in runaway beam behavior

NASA Astrophysics Data System (ADS)

Pankratov, I. M.; Zhou, R. J.; Hu, L. Q.

2015-07-01

Peculiar phenomena were observed during experiments with runaway electrons: rapid changes in the synchrotron spot and its intensity that coincided with stepwise increases in the electron cyclotron emission (ECE) signal (cyclotron radiation of suprathermal electrons). These phenomena were initially observed in TEXTOR (Tokamak Experiment for Technology Oriented Research), where these events only occurred in the current decay phase or in discharges with thin stable runaway beams at a q = 1 drift surface. These rapid changes in the synchrotron spot were interpreted by the TEXTOR team as a fast pitch angle scattering event. Recently, similar rapid changes in the synchrotron spot and its intensity that coincided with stepwise increases in the non-thermal ECE signal were observed in the EAST (Experimental Advanced Superconducting Tokamak) runaway discharge. Runaway electrons were located around the q = 2 rational magnetic surface (ring-like runaway electron beam). During the EAST runaway discharge, stepwise ECE signal increases coincided with enhanced magnetohydrodynamic (MHD) activity. This behavior was peculiar to this shot. In this paper, we show that these non-thermal ECE step-like jumps were related to the abrupt growth of suprathermal electrons induced by bursting electric fields at reconnection events during this MHD plasma activity. Enhancement of the secondary runaway electron generation also occurred simultaneously. Local changes in the current-density gradient appeared because of local enhancement of the runaway electron generation process. These current-density gradient changes are considered to be a possible trigger for enhancement of the MHD plasma activity and the rapid changes in runaway beam behavior.

Spectroscopic studies of the parameters of plasma jets during their propagation in the background plasma on the PF-3 facility

NASA Astrophysics Data System (ADS)

Dan'ko, S. A.; Ananyev, S. S.; Kalinin, Yu G.; Krauz, V. I.; Myalton, V. V.

2017-04-01

This paper presents measurement results of neon and helium plasma parameters in axial jets generated in plasma focus discharge. They were obtained in the course of experiments on laboratory modeling of astrophysical jets performed at the PF-3 facility. The plasma concentration was determined according to Stark broadening of spectral lines; the ionization temperature was determined by the average ion charge. The values of the concentration and temperature of jet plasma and background plasma at two distances from the pinch are also presented. In addition, an estimation was made of the heat content losses of the neon and helium jets during their movement through the surrounding medium.

Paper-based plasma sanitizers

NASA Astrophysics Data System (ADS)

Xie, Jingjin; Chen, Qiang; Suresh, Poornima; Roy, Subrata; White, James F.; Mazzeo, Aaron D.

2017-05-01

This work describes disposable plasma generators made from metallized paper. The fabricated plasma generators with layered and patterned sheets of paper provide a simple and flexible format for dielectric barrier discharge to create atmospheric plasma without an applied vacuum. The porosity of paper allows gas to permeate its bulk volume and fuel plasma, while plasma-induced forced convection cools the substrate. When electrically driven with oscillating peak-to-peak potentials of ±1 to ±10 kV, the paper-based devices produced both volume and surface plasmas capable of killing microbes. The plasma sanitizers deactivated greater than 99% of Saccharomyces cerevisiae and greater than 99.9% of Escherichia coli cells with 30 s of noncontact treatment. Characterization of plasma generated from the sanitizers revealed a detectable level of UV-C (1.9 nWṡcm-2ṡnm-1), modest surface temperature (60 °C with 60 s of activation), and a high level of ozone (13 ppm with 60 s of activation). These results deliver insights into the mechanisms and suitability of paper-based substrates for active antimicrobial sanitization with scalable, flexible sheets. In addition, this work shows how paper-based generators are conformable to curved surfaces, appropriate for kirigami-like “stretchy” structures, compatible with user interfaces, and suitable for sanitization of microbes aerosolized onto a surface. In general, these disposable plasma generators represent progress toward biodegradable devices based on flexible renewable materials, which may impact the future design of protective garments, skin-like sensors for robots or prosthetics, and user interfaces in contaminated environments.

Paper-based plasma sanitizers.

PubMed

Xie, Jingjin; Chen, Qiang; Suresh, Poornima; Roy, Subrata; White, James F; Mazzeo, Aaron D

2017-05-16

This work describes disposable plasma generators made from metallized paper. The fabricated plasma generators with layered and patterned sheets of paper provide a simple and flexible format for dielectric barrier discharge to create atmospheric plasma without an applied vacuum. The porosity of paper allows gas to permeate its bulk volume and fuel plasma, while plasma-induced forced convection cools the substrate. When electrically driven with oscillating peak-to-peak potentials of ±1 to ±10 kV, the paper-based devices produced both volume and surface plasmas capable of killing microbes. The plasma sanitizers deactivated greater than 99% of Saccharomyces cerevisiae and greater than 99.9% of Escherichia coli cells with 30 s of noncontact treatment. Characterization of plasma generated from the sanitizers revealed a detectable level of UV-C (1.9 nW⋅cm -2 ⋅nm -1 ), modest surface temperature (60 °C with 60 s of activation), and a high level of ozone (13 ppm with 60 s of activation). These results deliver insights into the mechanisms and suitability of paper-based substrates for active antimicrobial sanitization with scalable, flexible sheets. In addition, this work shows how paper-based generators are conformable to curved surfaces, appropriate for kirigami-like "stretchy" structures, compatible with user interfaces, and suitable for sanitization of microbes aerosolized onto a surface. In general, these disposable plasma generators represent progress toward biodegradable devices based on flexible renewable materials, which may impact the future design of protective garments, skin-like sensors for robots or prosthetics, and user interfaces in contaminated environments.

Recent advances in plasma devices based on plasma lens configuration for manipulating high-current heavy ion beams.

PubMed

Dobrovolskiy, A; Dunets, S; Evsyukov, A; Goncharov, A; Gushenets, V; Litovko, I; Oks, E

2010-02-01

We describe new results of development of novel generation cylindrical plasma devices based on the electrostatic plasma lens configuration and concept of electrons magnetic insulation. The crossed electric and magnetic fields plasma lens configuration provides us with the attractive and suitable method for establishing a stable plasma discharge at low pressure. Using plasma lens configuration in this way some cost-effective plasma devices were developed for ion treatment and deposition of exotic coatings and the effective lens was first proposed for manipulating high-current beams of negatively charged particles. Here we describe operation and features of these plasma devices, and results of theoretical consideration of mechanisms determining their optimal operation conditions.

Plasma ignition and steady state simulations of the Linac4 H- ion source

NASA Astrophysics Data System (ADS)

Mattei, S.; Ohta, M.; Yasumoto, M.; Hatayama, A.; Lettry, J.; Grudiev, A.

2014-02-01

The RF heating of the plasma in the Linac4 H- ion source has been simulated using a particle-in-cell Monte Carlo collision method. This model is applied to investigate the plasma formation starting from an initial low electron density of 1012 m-3 and its stabilization at 1018 m-3. The plasma discharge at low electron density is driven by the capacitive coupling with the electric field generated by the antenna, and as the electron density increases the capacitive electric field is shielded by the plasma and induction drives the plasma heating process. Plasma properties such as e-/ion densities and energies, sheath formation, and shielding effect are presented and provide insight to the plasma properties of the hydrogen plasma.

Thermal blanket metallic film groundstrap and second surface mirror vulnerability to arc discharges

NASA Technical Reports Server (NTRS)

Inouye, G. T.; Sanders, N. L.; Komatsu, G. K.; Valles, J. R.; Sellen, J. M., Jr.

1979-01-01

Available data on the geosynchronous orbit energetic plasma environment were examined, and a crude model was generated to permit an estimation to be made of the number of arc discharges per year to which a thermal blanket groundstrap would be subjected. Laboratory experiments and a survey of the literature on arc discharge characteristics were performed to define typical and worst case arc discharge current waveforms. In-air tests of different groundstrap configurations to a standardized test pulse were performed and a wide variability of durability values were found. A groundstrap technique, not used thus far, was found to be far superior than the others.

H- Ion Sources for High Intensity Proton Drivers

DOE Office of Scientific and Technical Information (OSTI.GOV)

Johnson, Rolland Paul; Dudnikov, Vadim

2015-02-20

Existing RF Surface Plasma Sources (SPS) for accelerators have specific efficiencies for H + and H - ion generation around 3 to 5 mA/cm 2 per kW, where about 50 kW of RF power is typically needed for 50 mA beam current production. The Saddle Antenna (SA) SPS described here was developed to improve H- ion production efficiency, reliability and availability for pulsed operation as used in the ORNL Spallation Neutron Source . At low RF power, the efficiency of positive ion generation in the plasma has been improved to 200 mA/cm 2 per kW of RF power at 13.56more » MHz. Initial cesiation of the SPS was performed by heating cesium chromate cartridges by discharge as was done in the very first versions of the SPS. A small oven to decompose cesium compounds and alloys was developed and tested. After cesiation, the current of negative ions to the collector was increased from 1 mA to 10 mA with RF power 1.5 kW in the plasma (6 mm diameter emission aperture) and up to 30 mA with 4 kW RF power in the plasma and 250 Gauss longitudinal magnetic field. The ratio of electron current to negative ion current was improved from 30 to 2. Stable generation of H- beam without intensity degradation was demonstrated in the aluminum nitride (AlN) discharge chamber for 32 days at high discharge power in an RF SPS with an external antenna. Some modifications were made to improve the cooling and cesiation stability. The extracted collector current can be increased significantly by optimizing the longitudinal magnetic field in the discharge chamber. While this project demonstrated the advantages of the pulsed version of the SA RF SPS as an upgrade to the ORNL Spallation Neutron Source, it led to a possibility for upgrades to CW machines like the many cyclotrons used for commercial applications. Four appendices contain important details of the work carried out under this grant.« less

Influence of High Speed Repetition of Pulsed Streamer Discharge Produced by Polarity-Reversed Traveling Wave on NO Oxidation

NASA Astrophysics Data System (ADS)

Matsuda, Eiji; Kadowaki, Kazunori; Nishimoto, Sakae; Kitani, Isamu

This paper describes experimental results of NO removal from a simulated exhausted gas using a barrier-type plasma reactor subjected to reciprocal traveling wave voltage pulses. A pulse-forming cable was charged and then grounded at one end without any resistance, so that a traveling wave reciprocated along the cable with a change in its polarity because the traveling wave was negatively reflected at the grounded-end. Transient discharge light between point-plane electrodes with a glass barrier was observed using a gated image-intensifier. Photographs of the transient discharge light indicated that many streamer channels extended widely in the gap at the initial stage in the voltage oscillation, while only an intense discharge channel was observed at the latter stage. NO removal tests were carried out using the reciprocal pulse generator and a coaxial plasma reactor with a cylindrical glass-barrier. Results indicated that the discharges at the first and the second polarity reversals contributed largely to the oxidation reaction from NO into NO2, whereas the contribution of the subsequent discharges in the latter stage to NO removal was small.

Plasma discharge elemental detector for a mass spectrometer

NASA Astrophysics Data System (ADS)

Heppner, R. A.

1983-06-01

A material to be analyzed is injected into a mirowave-induced plasma discharge unit, in which the material is carried with a flow of buffer gas through an intense microwave energy field which produces a plasma discharge in the buffer gas. As the material exits from the plasma discharge, the material is sampled and conveyed along a capillary transfer tube to a mass spectrometer where it is analyzed. The plasma discharge causes dissociation of complex organic molecules into simpler molecules which return to the neutral ground state before they are analyzed in the mass spectrometer. The buffer gas is supplied to one end portion of the discharge tube and is withdrawn from the other end portion by a vacuum pump which maintains a subatmospheric pressure in the discharge tube. The sample material is injected by a capillary injection tube into the buffer gas flow as it enters the plasma discharge zone. The dissociated materials are sampled by an axial sampling tube having an entrance where the buffer gas exits from the plasma discharge zone. The sample material may be supplied by a gas chromatography having a capillary effluent line connected to the capillary injection tube, so that the effluent material is injected into the microwave induced plasma discharge. The microwave field is produced by a cavity resonator through which the discharge tube passes.

Radio-Frequency Plasma Cleaning of a Penning Malmberg Trap

NASA Technical Reports Server (NTRS)

Sims, William Herbert, III; Martin, James; Pearson, J. Boise; Lewis, Raymond

2005-01-01

Radio-frequency-generated plasma has been demonstrated to be a promising means of cleaning the interior surfaces of a Penning-Malmberg trap that is used in experiments on the confinement of antimatter. {Such a trap was reported in Modified Penning-Malmberg Trap for Storing Antiprotons (MFS-31780), NASA Tech Briefs, Vol. 29, No. 3 (March 2005), page 66.} Cleaning of the interior surfaces is necessary to minimize numbers of contaminant atoms and molecules, which reduce confinement times by engaging in matter/antimatter-annihilation reactions with confined antimatter particles. A modified Penning-Malmberg trap like the one described in the cited prior article includes several collinear ring electrodes (some of which are segmented) inside a tubular vacuum chamber, as illustrated in Figure 1. During operation of the trap, a small cloud of charged antiparticles (e.g., antiprotons or positrons) is confined to a spheroidal central region by means of a magnetic field in combination with DC and radiofrequency (RF) electric fields applied via the electrodes. In the present developmental method of cleaning by use of RF-generated plasma, one evacuates the vacuum chamber, backfills the chamber with hydrogen at a suitable low pressure, and uses an RF-signal generator and baluns to apply RF voltages to the ring electrodes. Each ring is excited in the polarity opposite that of the adjacent ring. The electric field generated by the RF signal creates a discharge in the low-pressure gas. The RF power and gas pressure are adjusted so that the plasma generated in the discharge (see Figure 2) physically and chemically attacks any solid, liquid, and gaseous contaminant layers on the electrode surfaces. The products of the physical and chemical cleaning reactions are gaseous and are removed by the vacuum pumps.

Generation of high charge state metal ion beams by electron cyclotron resonance heating of vacuum arc plasma in cusp trap.

PubMed

Nikolaev, A G; Savkin, K P; Oks, E M; Vizir, A V; Yushkov, G Yu; Vodopyanov, A V; Izotov, I V; Mansfeld, D A

2012-02-01

A method for generating high charge state heavy metal ion beams based on high power microwave heating of vacuum arc plasma confined in a magnetic trap under electron cyclotron resonance conditions has been developed. A feature of the work described here is the use of a cusp magnetic field with inherent "minimum-B" structure as the confinement geometry, as opposed to a simple mirror device as we have reported on previously. The cusp configuration has been successfully used for microwave heating of gas discharge plasma and extraction from the plasma of highly charged, high current, gaseous ion beams. Now we use the trap for heavy metal ion beam generation. Two different approaches were used for injecting the vacuum arc metal plasma into the trap--axial injection from a miniature arc source located on-axis near the microwave window, and radial injection from sources mounted radially at the midplane of the trap. Here, we describe preliminary results of heating vacuum arc plasma in a cusp magnetic trap by pulsed (400 μs) high power (up to 100 kW) microwave radiation at 37.5 GHz for the generation of highly charged heavy metal ion beams.

An university-scale pulsed-power system using a bipolar Marx generator

NASA Astrophysics Data System (ADS)

Chang, Po-Yu; Yang, Sheng-Hua; Huang, Mei-Feng; Isaps, Natl Cheng Kung Univ Team

2017-10-01

A bipolar Marx generator is being built for x-ray sources or laboratory astrophysics and space research for university-scale laboratory. The system consists of ten stages. In each stage, two 1 μF capacitors connected in series are charged to +/- 30 kV storing 9 kJ of total energy. It delivers a current of 200 kA to the load with a 200 ns rise time during the discharge. It will be used for following three purposes: (1) gas-puff z pinches generating soft x-ray for bio-medical research in the future; (2) generating plasma jets to study interactions between plasma flows and unmagnetized/magnetized obstacles analogous to the interactions between solar winds and planetary magnetic fields or unmagnetized planets; and (3) studying the pinch in a dense plasma focus device. The results of current measurements and circuit characteristics are shown.

Variation in structure of proteins by adjusting reactive oxygen and nitrogen species generated from dielectric barrier discharge jet

NASA Astrophysics Data System (ADS)

Park, Ji Hoon; Kim, Minsup; Shiratani, Masaharu; Cho, Art. E.; Choi, Eun Ha; Attri, Pankaj

2016-10-01

Over the last few years, the variation in liquid chemistry due to the development of radicals generated by cold atmospheric plasma (CAP) has played an important role in plasma medicine. CAP direct treatment or CAP activated media treatment in cancer cells shows promising anticancer activity for both in vivo and in vitro studies. However, the anticancer activity or antimicrobial activity varies between plasma devices due to the different abilities among plasma devices to generate the reactive oxygen and nitrogen species (RONS) at different ratios and in different concentrations. While the generation of RONS depends on many factors, the feeding gas plays the most important role among the factors. Hence, in this study we used different compositions of feeding gas while fixing all other plasma characteristics. We used Ar, Ar-O2 (at different ratios), and Ar-N2 (at different ratios) as the working gases for CAP and investigated the structural changes in proteins (Hemoglobin (Hb) and Myoglobin (Mb)). We then analyzed the influence of RONS generated in liquid on the conformations of proteins. Additionally, to determine the influence of H2O2 on the Hb and Mb structures, we used molecular dynamic simulation.

Thrust performance, propellant ionization, and thruster erosion of an external discharge plasma thruster

NASA Astrophysics Data System (ADS)

Karadag, Burak; Cho, Shinatora; Funaki, Ikkoh

2018-04-01

It is quite a challenge to design low power Hall thrusters with a long lifetime and high efficiency because of the large surface area to volume ratio and physical limits to the magnetic circuit miniaturization. As a potential solution to this problem, we experimentally investigated the external discharge plasma thruster (XPT). The XPT produces and sustains a plasma discharge completely in the open space outside of the thruster structure through a magnetic mirror configuration. It eliminates the very fundamental component of Hall thrusters, discharge channel side walls, and its magnetic circuit consists solely of a pair of hollow cylindrical permanent magnets. Thrust, low frequency discharge current oscillation, ion beam current, and plasma property measurements were conducted to characterize the manufactured prototype thruster for the proof of concept. The thrust performance, propellant ionization, and thruster erosion were discussed. Thrust generated by the XPT was on par with conventional Hall thrusters [stationary plasma thruster (SPT) or thruster with anode layer] at the same power level (˜11 mN at 250 W with 25% anode efficiency without any optimization), and discharge current had SPT-level stability (Δ < 0.2). Faraday probe measurements revealed that ion beams are finely collimated, and plumes have Gaussian distributions. Mass utilization efficiencies, beam utilization efficiencies, and plume divergence efficiencies ranged from 28 to 62%, 78 to 99%, and 40 to 48%, respectively. Electron densities and electron temperatures were found to reach 4 × 1018 m-3 ( ∂ n e / n e = ±52%) and 15 eV ( ∂ T e / T e = ±10%-30%), respectively, at 10 mm axial distance from the anode centerline. An ionization mean free path analysis revealed that electron density in the ionization region is substantially higher than the conventional Hall thrusters, which explain why the XPT is as efficient as conventional ones even without a physical ionization chamber. Our findings propose an alternative approach for low power Hall thruster design and provide a successful proof of concept experiment of the XPT.

Nitric oxide kinetics in the afterglow of a diffuse plasma filament

NASA Astrophysics Data System (ADS)

Burnette, D.; Montello, A.; Adamovich, I. V.; Lempert, W. R.

2014-08-01

A suite of laser diagnostics is used to study kinetics of vibrational energy transfer and plasma chemical reactions in a nanosecond pulse, diffuse filament electric discharge and afterglow in N2 and dry air at 100 Torr. Laser-induced fluorescence of NO and two-photon absorption laser-induced fluorescence of O and N atoms are used to measure absolute, time-resolved number densities of these species after the discharge pulse, and picosecond coherent anti-Stokes Raman spectroscopy is used to measure time-resolved rotational temperature and ground electronic state N2(v = 0-4) vibrational level populations. The plasma filament diameter, determined from plasma emission and NO planar laser-induced fluorescence images, remains nearly constant after the discharge pulse, over a few hundred microseconds, and does not exhibit expansion on microsecond time scale. Peak temperature in the discharge and the afterglow is low, T ≈ 370 K, in spite of significant vibrational nonequilibrium, with peak N2 vibrational temperature of Tv ≈ 2000 K. Significant vibrational temperature rise in the afterglow is likely caused by the downward N2-N2 vibration-vibration (V-V) energy transfer. Simple kinetic modeling of time-resolved N, O, and NO number densities in the afterglow, on the time scale longer compared to relaxation and quenching time of excited species generated in the plasma, is in good agreement with the data. In nitrogen, the N atom density after the discharge pulse is controlled by three-body recombination and radial diffusion. In air, N, NO and O concentrations are dominated by the reverse Zel'dovich reaction, N + NO → N2 + O, and ozone formation reaction, O + O2 + M → O3 + M, respectively. The effect of vibrationally excited nitrogen molecules and excited N atoms on NO formation kinetics is estimated to be negligible. The results suggest that NO formation in the nanosecond pulse discharge is dominated by reactions of excited electronic states of nitrogen, occurring on microsecond time scale.

Power matching between plasma generation and electrostatic acceleration in helicon electrostatic thruster

NASA Astrophysics Data System (ADS)

Ichihara, D.; Nakagawa, Y.; Uchigashima, A.; Iwakawa, A.; Sasoh, A.; Yamazaki, T.

2017-10-01

The effects of a radio-frequency (RF) power on the ion generation and electrostatic acceleration in a helicon electrostatic thruster were investigated with a constant discharge voltage of 300 V using argon as the working gas at a flow rate either of 0.5 Aeq (Ampere equivalent) or 1.0 Aeq. A RF power that was even smaller than a direct-current (DC) discharge power enhanced the ionization of the working gas, thereby both the ion beam current and energy were increased. However, an excessively high RF power input resulted in their saturation, leading to an unfavorable increase in an ionization cost with doubly charged ion production being accompanied. From the tradeoff between the ion production by the RF power and the electrostatic acceleration made by the direct current discharge power, the thrust efficiency has a maximum value at an optimal RF to DC discharge power ratio of 0.6 - 1.0.

Modeling and characterization of field-enhanced corona discharge in ozone-generator diode

NASA Astrophysics Data System (ADS)

Patil, Jagadish G.; Vijayan, T.

2010-02-01

Electric field enhanced corona plasma discharge in ozone generator diode of axial symmetry has been investigated and characterized in theory. The cathode K of diode is made of a large number of sharpened nozzles arranged on various radial planes on the axial mast and pervaded in oxygen gas inside the anode cup A, produces high fields over MV/m and aids in the formation of a corona plume of dense ozone cloud over the cathode surface. An r-z finite difference scheme has been devised and employed to numerically determine the potential and electric field distributions inside the diode. The analyses of cathode emissions revealed a field emission domain conformed to modified Child-Langmuir diode-current. Passage of higher currents (over μA) in shorter A-K gaps d gave rise to cathode heated plasma extending from the corona to Saha regimes depending on local temperature. Plasma densities of order 102-106 m-3 are predicted in these. For larger d however, currents are smaller and heating negligible and a negative corona favoring ozone formation is attained. High ozone yields about 20 per cent of oxygen input is predicted in this domain. The generator so developed will be applied to various important applications such as, purification of ambient air /drinking water, ozone therapy, and so on.

Plasma characterization of the superconducting proton linear accelerator plasma generator using a 2 MHz compensated Langmuir probe.

PubMed

Schmitzer, C; Kronberger, M; Lettry, J; Sanchez-Arias, J; Störi, H

2012-02-01

The CERN study for a superconducting proton Linac (SPL) investigates the design of a pulsed 5 GeV Linac operating at 50 Hz. As a first step towards a future SPL H(-) volume ion source, a plasma generator capable of operating at Linac4 or nominal SPL settings has been developed and operated at a dedicated test stand. The hydrogen plasma is heated by an inductively coupled RF discharge e(-) and ions are confined by a magnetic multipole cusp field similar to the currently commissioned Linac4 H(-) ion source. Time-resolved measurements of the plasma potential, temperature, and electron energy distribution function obtained by means of a RF compensated Langmuir probe along the axis of the plasma generator are presented. The influence of the main tuning parameters, such as RF power and frequency and the timing scheme is discussed with the aim to correlate them to optimum H(-) ion beam parameters measured on an ion source test stand. The effects of hydrogen injection settings which allow operation at 50 Hz repetition rate are discussed.

Plasma characterization of the superconducting proton linear accelerator plasma generator using a 2 MHz compensated Langmuir probea)

NASA Astrophysics Data System (ADS)

Schmitzer, C.; Kronberger, M.; Lettry, J.; Sanchez-Arias, J.; Störi, H.

2012-02-01

The CERN study for a superconducting proton Linac (SPL) investigates the design of a pulsed 5 GeV Linac operating at 50 Hz. As a first step towards a future SPL H- volume ion source, a plasma generator capable of operating at Linac4 or nominal SPL settings has been developed and operated at a dedicated test stand. The hydrogen plasma is heated by an inductively coupled RF discharge e- and ions are confined by a magnetic multipole cusp field similar to the currently commissioned Linac4 H- ion source. Time-resolved measurements of the plasma potential, temperature, and electron energy distribution function obtained by means of a RF compensated Langmuir probe along the axis of the plasma generator are presented. The influence of the main tuning parameters, such as RF power and frequency and the timing scheme is discussed with the aim to correlate them to optimum H- ion beam parameters measured on an ion source test stand. The effects of hydrogen injection settings which allow operation at 50 Hz repetition rate are discussed.

Reactive species in non-equilibrium atmospheric-pressure plasmas: Generation, transport, and biological effects

NASA Astrophysics Data System (ADS)

Lu, X.; Naidis, G. V.; Laroussi, M.; Reuter, S.; Graves, D. B.; Ostrikov, K.

2016-05-01

Non-equilibrium atmospheric-pressure plasmas have recently become a topical area of research owing to their diverse applications in health care and medicine, environmental remediation and pollution control, materials processing, electrochemistry, nanotechnology and other fields. This review focuses on the reactive electrons and ionic, atomic, molecular, and radical species that are produced in these plasmas and then transported from the point of generation to the point of interaction with the material, medium, living cells or tissues being processed. The most important mechanisms of generation and transport of the key species in the plasmas of atmospheric-pressure plasma jets and other non-equilibrium atmospheric-pressure plasmas are introduced and examined from the viewpoint of their applications in plasma hygiene and medicine and other relevant fields. Sophisticated high-precision, time-resolved plasma diagnostics approaches and techniques are presented and their applications to monitor the reactive species and plasma dynamics in the plasma jets and other discharges, both in the gas phase and during the plasma interaction with liquid media, are critically reviewed. The large amount of experimental data is supported by the theoretical models of reactive species generation and transport in the plasmas, surrounding gaseous environments, and plasma interaction with liquid media. These models are presented and their limitations are discussed. Special attention is paid to biological effects of the plasma-generated reactive oxygen and nitrogen (and some other) species in basic biological processes such as cell metabolism, proliferation, survival, etc. as well as plasma applications in bacterial inactivation, wound healing, cancer treatment and some others. Challenges and opportunities for theoretical and experimental research are discussed and the authors' vision for the emerging convergence trends across several disciplines and application domains is presented to stimulate critical discussions and collaborations in the future.

Dynamics of ion beam charge neutralization by ferroelectric plasma sources

DOE PAGES

Stepanov, Anton D.; Gilson, Erik P.; Grisham, Larry R.; ...

2016-04-27

Ferroelectric Plasma Sources (FEPSs) can generate plasma that provides effective space-charge neutralization of intense high-perveance ion beams, as has been demonstrated on the Neutralized Drift Compression Experiment NDCX-I and NDCX-II. This article presents experimental results on charge neutralization of a high-perveance 38 keV Ar + beam by a plasma produced in a FEPS discharge. By comparing the measured beam radius with the envelope model for space-charge expansion, it is shown that a charge neutralization fraction of 98% is attainable with sufficiently dense FEPS plasma. The transverse electrostatic potential of the ion beam is reduced from 15V before neutralization to 0.3more » V, implying that the energy of the neutralizing electrons is below 0.3 eV. Measurements of the time-evolution of beam radius show that near-complete charge neutralization is established similar to –5 μs after the driving pulse is applied to the FEPS and can last for 35 μs. It is argued that the duration of neutralization is much longer than a reasonable lifetime of the plasma produced in the sub-mu s surface discharge. Measurements of current flow in the driving circuit of the FEPS show the existence of electron emission into vacuum, which lasts for tens of mu s after the high voltage pulse is applied. Lastly, it is argued that the beam is neutralized by the plasma produced by this process and not by a surface discharge plasma that is produced at the instant the high-voltage pulse is applied.« less

Characteristics of a Direct Current-driven plasma jet operated in open air

NASA Astrophysics Data System (ADS)

Li, Xuechen; Di, Cong; Jia, Pengying; Bao, Wenting

2013-09-01

A DC-driven plasma jet has been developed to generate a diffuse plasma plume by blowing argon into the ambient air. The plasma plume, showing a cup shape with a diameter of several centimeters at a higher voltage, is a pulsed discharge despite a DC voltage is applied. The pulse frequency is investigated as a function of the voltage under different gap widths and gas flow rates. Results show that plasma bullets propagate from the hollow needle to the plate electrode by spatially resolved measurement. A supposition about non-electroneutral trail of the streamer is proposed to interpret these experimental phenomena.

Irradiation of orderly multiline spectra from linear plasma formed by vacuum discharge capillary

NASA Astrophysics Data System (ADS)

Sato, Eiichi; Hayasi, Yasuomi; Germer, Rudolf; Ojima, Hidenori; Takayama, Kazuyoshi; Ido, Hideaki

2005-03-01

The fundamental experiments for measuring soft x-ray characteristics from the vacuum capillary are described. These experiments are primarily performed in order to generate intense soft x rays. The generator consists of a high-voltage power supply, a polarity-inversion ignitron pulse generator, a turbomolecular pump, and a radiation tube with a capillary. A high-voltage condenser of 200 nF in the pulse generator is charged up to 20 kV by the power supply, and the electric charges in the condenser are discharged to the capillary in the tube after closing the ignitron. During the discharge, weakly ionized plasma forms on the inner and outer sides of a capillary. In the present work, the pump evacuates air from the tube with a pressure of about 1 mPa, and a demountable capillary was developed in order to measure x-ray spectra according to changes in the capillary length. In this capillary, the anode (target) and cathode elements can be changed corresponding to the objectives. The capillary diameter is 2.0 mm, and the length is adjusted from 1 to 50 mm. When a capillary with aluminum anode and cathode electrodes was employed, both the cathode voltage and the discharge current almost displayed damped oscillations. The peak values of the voltage and current increased when the charging voltage was increased, and their maximum values were -11.5 kV and 4.7 kA, respectively. The x-ray durations observed by a 1.6 μm aluminum filter were less than 30 μs. In the spectrum measurement, we observed orderly multi-line spectra. The line photon energies seldom varied according to changes in the condenser charging voltage and to changes in the electrode element. The line number decreased with corresponding decreases in the capillary length.

Formation of hydrophobic coating on glass surface using atmospheric pressure non-thermal plasma in ambient air

NASA Astrophysics Data System (ADS)

Fang, Z.; Qiu, Y.; Kuffel, E.

2004-08-01

Non-thermal plasmas under atmospheric pressure are of great interest in material surface processing because of their convenience, effectiveness and low cost. In this paper, the treatment of a glass surface for improving hydrophobicity using a non-thermal plasma generated by a dielectric barrier corona discharge (DBCD) with a needle array-to-plane electrode arrangement in atmospheric air is conducted, and the surface properties of the glass before and after the DBCD treatment are studied using contact angle measurement, surface resistance measurement and the wet flashover voltage test. The effects of the plasma dose (the product of average discharge power and treatment time) of DBCD on the surface modification are studied, and the mechanism of interaction between the plasma and glass surface is discussed. It is found that a layer of hydrophobic coating is formed on the glass surface through DBCD treatment, and the improvement of hydrophobicity depends on the plasma dose of the DBCD. It seems that there is an optimum plasma dose for the surface treatment. The test results of thermal ageing and chemical ageing show that the hydrophobic layer has quite stable characteristics.

Large-aperture Tunable Plasma Meta-material to Interact with Electromagnetic Waves

NASA Astrophysics Data System (ADS)

Corke, Thomas; Matlis, Eric

2016-11-01

The formation of spatially periodic arrangements of glow discharge plasma resulting from charge instabilities were investigated as a tuneable plasma meta-material. The plasma was formed between two 2-D parallel dielectric covered electrodes: one consisting of an Indium-Tin-Oxide coated glass sheet, and the other consisting of a glass-covered circular electrode. The dielectric covered electrodes were separated by a gap that formed a 2-D channel. The gap spacing was adjustable. The electrodes were powered by a variable amplitude AC generator. The parallel electrode arrangement was placed in a variable pressure vacuum chamber. Various combinations of gap spacing, pressure and voltage resulted in the formation of spatially periodic arrangements (lattice) of glow discharge plasma. The lattice spacing perfectly followed 2-D packing theory, and was fully adjustable through the three governing parameters. Lattice arrangements were designed to interact with electromagnetic (EM) waves in the frequency range between 10GHz-80GHz. Its feasibility was investigate through an EM wave simulation that we adapted to allow for plasma permittivity. The results showed a clear suppression of the EM wave amplitude through the plasma gratings. Supported by AFOSR.

Plasma x-ray radiation source.

PubMed

Popkov, N F; Kargin, V I; Ryaslov, E A; Pikar', A S

1995-01-01

This paper gives the results of studies on a plasma x-ray source, which enables one to obtain a 2.5-krad radiation dose per pulse over an area of 100 cm2 in the quantum energy range from 20 to 500 keV. Pulse duration is 100 ns. Spectral radiation distributions from a diode under various operation conditions of a plasma are obtained. A Marx generator served as an initial energy source of 120 kJ with a discharge time of T/4 = 10-6 s. A short electromagnetic pulse (10-7 s) was shaped using plasma erosion opening switches.

An amplitude modulated radio frequency plasma generator

NASA Astrophysics Data System (ADS)

Lei, Fan; Li, Xiaoping; Liu, Yanming; Liu, Donglin; Yang, Min; Xie, Kai; Yao, Bo

2017-04-01

A glow discharge plasma generator and diagnostic system has been developed to study the effects of rapidly variable plasmas on electromagnetic wave propagation, mimicking the plasma sheath conditions encountered in space vehicle reentry. The plasma chamber is 400 mm in diameter and 240 mm in length, with a 300-mm-diameter unobstructed clear aperture. Electron densities produced are in the mid 1010 electrons/cm3. An 800 W radio frequency (RF) generator is capacitively coupled through an RF matcher to an internally cooled stainless steel electrode to form the plasma. The RF power is amplitude modulated by a waveform generator that operates at different frequencies. The resulting plasma contains electron density modulations caused by the varying power levels. A 10 GHz microwave horn antenna pair situated on opposite sides of the chamber serves as the source and detector of probe radiation. The microwave power feed to the source horn is split and one portion is sent directly to a high-speed recording oscilloscope. On mixing this with the signal from the pickup horn antenna, the plasma-induced phase shift between the two signals gives the path-integrated electron density with its complete time dependent variation. Care is taken to avoid microwave reflections and extensive shielding is in place to minimize electronic pickup. Data clearly show the low frequency modulation of the electron density as well as higher harmonics and plasma fluctuations.

Plasma Discharges in Gas Bubbles in Liquid Water: Breakdown Mechanisms and Resultant Chemistry

NASA Astrophysics Data System (ADS)

Gucker, Sarah M. N.

The use of atmospheric pressure plasmas in gases and liquids for purification of liquids has been investigated by numerous researchers, and is highly attractive due to their strong potential as a disinfectant and sterilizer. However, the fundamental understanding of plasma production in liquid water is still limited. Despite the decades of study dedicated to electrical discharges in liquids, many physical aspects of liquids, such as the high inhomogeneity of liquids, complicate analyses. For example, the complex nonlinearities of the fluid have intricate effects on the electric field of the propagating streamer. Additionally, the liquid material itself can vaporize, leading to discontinuous liquid-vapor boundaries. Both can and do often lead to notable hydrodynamic effects. The chemistry of these high voltage discharges on liquid media can have circular effects, with the produced species having influence on future discharges. Two notable examples include an increase in liquid conductivity via charged species production, which affects the discharge. A second, more complicated scenario seen in some liquids (such as water) is the doubling or tripling of molecular density for a few molecule layers around a high voltage electrode. These complexities require technological advancements in optical diagnostics that have only recently come into being. This dissertation investigates several aspects of electrical discharges in gas bubbles in liquids. Two primary experimental configurations are investigated: the first allows for single bubble analysis through the use of an acoustic trap. Electrodes may be brought in around the bubble to allow for plasma formation without physically touching the bubble. The second experiment investigates the resulting liquid phase chemistry that is driven by the discharge. This is done through a dielectric barrier discharge with a central high voltage surrounded by a quartz discharge tube with a coil ground electrode on the outside. The plasma is created either through flowing gas around the high voltage electrode in the discharge tube or self-generated by the plasma as in the steam discharge. This second method allows for large scale processing of contaminated water and for bulk chemical and optical analysis. Breakdown mechanisms of attached and unattached gas bubbles in liquid water were investigated using the first device. The breakdown scaling relation between breakdown voltage, pressure and dimensions of the discharge was studied. A Paschen-like voltage dependence for air bubbles in liquid water was discovered. The results of high-speed photography suggest the physical charging of the bubble due to a high voltage pulse; this charging can be significant enough to produce rapid kinetic motion of the bubble about the electrode region as the applied electric field changes over a voltage pulse. Physical deformation of the bubble is observed. This charging can also prevent breakdown from occurring, necessitating higher applied voltages to overcome the phenomenon. This dissertation also examines the resulting chemistry from plasma interacting with the bubble-liquid system. Through the use of optical emission spectroscopy, plasma parameters such as electron density, gas temperature, and molecular species production and intensity are found to have a time-dependence over the ac voltage cycle. This dependence is also source gas type dependent. These dependencies afford effective control over plasma-driven decomposition. The effect of plasma-produced radicals on various wastewater simulants is studied. Various organic dyes, halogenated compounds, and algae water are decomposed and assessed. Toxicology studies with melanoma cells exposed to plasma-treated dye solutions are completed, demonstrating the non-cytotoxic quality of the decomposition process. Thirdly, this dissertation examines the steam plasma system, developed through this research to circumvent the acidification associated with gas-feed discharges. This steam plasma creates its own gas pocket via field emission. This steam plasma is shown to have strong decontamination properties, with residual effects lasting beyond two weeks that continue to decompose contaminants. Finally, a "two-dimensional bubble" was developed and demonstrated as a novel diagnostic device to study the gas-water interface, the reaction zone. This device is shown to provide convenient access to the reaction zone and decomposition of various wastewater simulants is investigated.

Pulsed electrical discharge in gas bubbles in water

NASA Astrophysics Data System (ADS)

Gershman, Sophia

A phenomenological picture of pulsed electrical discharge in gas bubbles in water is produced by combining electrical, spectroscopic, and imaging methods. The discharge is generated by applying one microsecond long 5 to 20 kilovolt pulses between the needle and disk electrodes submerged in water. A gas bubble is generated at the tip of the needle electrode. The study includes detailed experimental investigation of the discharge in argon bubbles and a brief look at the discharge in oxygen bubbles. Imaging, electrical characteristics, and time-resolved optical emission data point to a fast streamer propagation mechanism and formation of a plasma channel in the bubble. Spectroscopic methods based on line intensity ratios and Boltzmann plots of line intensities of argon, atomic hydrogen, and argon ions and the examination of molecular emission bands from molecular nitrogen and hydroxyl radicals provide evidence of both fast beam-like electrons and slow thermalized ones with temperatures of 0.6 -- 0.8 electron-volts. The collisional nature of plasma at atmospheric pressure affects the decay rates of optical emission. Spectroscopic study of rotational-vibrational bands of hydroxyl radical and molecular nitrogen gives vibrational and rotational excitation temperatures of the discharge of about 0.9 and 0.1 electron-volt, respectively. Imaging and electrical evidence show that discharge charge is deposited on the bubble wall and water serves as a dielectric barrier for the field strength and time scales of this experiment. Comparing the electrical and imaging information for consecutive pulses applied at a frequency of 1 Hz indicates that each discharge proceeds as an entirely new process with no memory of the previous discharge aside from long-lived chemical species, such as ozone and oxygen. Intermediate values for the discharge gap and pulse duration, low repetition rate, and unidirectional character of the applied voltage pulses make the discharge process here unique compared to the traditional corona or dielectric barrier discharges. These conditions make the experimental evidence presented in this work valuable for the advancement of modeling and the theoretical understanding of the discharge in bubbles in water.

Temporal response of a surface flashover on a velvet cathode in a relativistic diode

DOE Office of Scientific and Technical Information (OSTI.GOV)

Coleman, J. E.; Moir, D. C.; Crawford, M. T.

2015-03-15

Surface flashover of a carbon fiber velvet cathode generates a discharge from which electrons are relativistically accelerated to γ ranging from 4.9 to 8.8 through a 17.8 cm diode. This discharge is assumed to be a hydrocarbon mixture. The principal objective of these experiments is to quantify the dynamics over the ∼100 ns pulse of the plasma discharge generated on the surface of the velvet cathode and across the anode-cathode (A-K) gap. A qualitative comparison of calculated and measured results is presented, which includes time resolved measurements with a photomultiplier tube and charge-coupled device images. In addition, initial visible spectroscopy measurements willmore » also be presented confirming the ion species are dominated by hydrogen.« less

OH Production Enhancement in Bubbling Pulsed Discharges

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lungu, Cristian P.; Porosnicu, Corneliu; Jepu, Ionut

2010-10-13

The generation of active species, such as H{sub 2}O{sub 2}, O{sup *}, OH*, HO{sub 2}*, O{sub 3}, N{sub 2}{sup *}, etc, produced in aqueous solutions by HV pulsed discharges was studied in order to find the most efficient way in waste water treatment taking into account that these species are almost stronger oxidizers than ozone. Plasma was generated inside gas bubbles formed by the argon, air and oxygen gas flow between the special designed electrodes. The pulse width and pulse frequency influence was studied in order to increase the efficiency of the OH active species formation. The produced active speciesmore » were investigated by optical emission spectroscopy and correlated with electrical parameters of the discharges (frequency, pulse width, amplitude, and rise and decay time).« less

Experimental investigations of a uranium plasma pertinent to a self-sustaining plasma source

NASA Technical Reports Server (NTRS)

Schneider, R. T.

1971-01-01

The research is pertinent to the realization of a self-sustained fissioning plasma for applications such as nuclear propulsion, closed cycle MHD power generation using a plasma core reactor, and heat engines such as the nuclear piston engine, as well as the direct conversion of fission energy into optical radiation (nuclear pumped lasers). Diagnostic measurement methods and experimental devices simulating plasma core reactor conditions are discussed. Studies on the following topics are considered: (1) ballistic piston compressor (U-235); (2) high pressure uranium plasma (natural uranium); (3) sliding spark discharge (natural uranium); (4) fission fragment interaction (He-3 and U-235); and (5) nuclear pumped lasers (He-3 and U-235).

Process Properties of Electronic High Voltage Discharges Triggered by Ultra-short Pulsed Laser Filaments

NASA Astrophysics Data System (ADS)

Cvecek, Kristian; Gröschel, Benjamin; Schmidt, Michael

Remote processing of metallic workpieces by techniques based on electric arc discharge or laser irradiation for joining or cutting has a long tradition and is still being intensively investigated in present-day research. In applications that require high power processing, both approaches exhibit certain advantages and disadvantages that make them specific for a given task. While several hybrid approaches exist that try to combine the benefits of both techniques, none were as successful in providing a fixed electric discharge direction as discharges triggered by plasma filaments generated by ultra-short pulsed lasers. In this work we investigate spatial and temporal aspects of laser filament guided discharges and give an upper time delay between the filament creation and the electrical build-up of a dischargeable voltage for a successful filament triggered discharge.

Characterization of pulsed atmospheric-pressure plasma streams (PAPS) generated by a plasma gun

NASA Astrophysics Data System (ADS)

Robert, E.; Sarron, V.; Riès, D.; Dozias, S.; Vandamme, M.; Pouvesle, J.-M.

2012-06-01

An experimental study of atmospheric-pressure rare gas plasma propagation in a high-aspect-ratio capillary is reported. The plasma is generated with a plasma gun device based on a dielectric barrier discharge (DBD) reactor powered by either nanosecond or microsecond rise-time high-voltage pulses at single-shot to multi-kHz frequencies. The influence of the voltage waveform, pulse polarity, pulse repetition rate and capillary material have been studied using nanosecond intensified charge-coupled device imaging and plasma-front velocity measurements. The evolution of the plasma appearance during its propagation and the study of the role of the different experimental parameters lead us to suggest a new denomination of pulsed atmospheric-pressure plasma streams to describe all the plasma features, including the previously so-called plasma bullet. The unique properties of such non-thermal plasma launching in capillaries, far from the primary DBD plasma, are associated with a fast ionization wave travelling with velocity in the 107-108 cm s-1 range. Voltage pulse tailoring is shown to allow for a significant improvement of such plasma delivery. Thus, the plasma gun device affords unique opportunities in biomedical endoscopic applications.

Real-time imaging, spectroscopy, and structural investigation of cathodic plasma electrolytic oxidation of molybdenum

NASA Astrophysics Data System (ADS)

Stojadinović, Stevan; Tadić, Nenad; Šišović, Nikola M.; Vasilić, Rastko

2015-06-01

In this paper, the results of the investigation of cathodic plasma electrolytic oxidation (CPEO) of molybdenum at 160 V in a mixed solution of borax, water, and ethylene glycol are presented. Real-time imaging and optical emission spectroscopy were used for the characterization of the CPEO. During the process, vapor envelope is formed around the cathode and strong electric field within the envelope caused the generation of plasma discharges. The spectral line shape analysis of hydrogen Balmer line Hβ (486.13 nm) shows that plasma discharges are characterized by the electron number density of about 1.4 × 1021 m-3. The electron temperature of 15 000 K was estimated by measuring molybdenum atomic lines intensity. Surface morphology, chemical, and phase composition of coatings formed by CPEO were characterized by scanning electron microscopy with energy dispersive x-ray spectroscopy and x-ray diffraction. The elemental components of CPEO coatings are Mo and O and the predominant crystalline form is MoO3.

Apparatus and method for atmospheric pressure reactive atom plasma processing for shaping of damage free surfaces

DOEpatents

Carr,; Jeffrey, W [Livermore, CA

2009-03-31

Fabrication apparatus and methods are disclosed for shaping and finishing difficult materials with no subsurface damage. The apparatus and methods use an atmospheric pressure mixed gas plasma discharge as a sub-aperture polisher of, for example, fused silica and single crystal silicon, silicon carbide and other materials. In one example, workpiece material is removed at the atomic level through reaction with fluorine atoms. In this example, these reactive species are produced by a noble gas plasma from trace constituent fluorocarbons or other fluorine containing gases added to the host argon matrix. The products of the reaction are gas phase compounds that flow from the surface of the workpiece, exposing fresh material to the etchant without condensation and redeposition on the newly created surface. The discharge provides a stable and predictable distribution of reactive species permitting the generation of a predetermined surface by translating the plasma across the workpiece along a calculated path.

Experimental Study on Inactivation of Bacterial Endotoxin by Using Dielectric Barrier Discharge

NASA Astrophysics Data System (ADS)

Shi, Xingmin; Li, Yaxi; Zhang, Guanjun; Ma, Yue; Shao, Xianjun

2011-12-01

The low-temperature plasma (LTP) generated by dielectric barrier discharge (DBD) was used to sterilize the E.coli endotoxin, which is usually difficult to kill by traditional methods. Three different concentrations of bacterial endotoxin (1 EU/mL, 0.5 EU/mL and 0.25 EU/mL) were treated by LTP for different time (20 s, 40 s and 60 s). Tachypleus amebocyte lysate (TAL) method was employed to detect the concentration variation of bacterial endotoxin before and after the plasma treatment, and endotoxic shock mice model was used to evaluate the inactivation effects of LTP on endotoxin for further study. Experimental results demonstrated that, DBD plasma can inactivate the bacterial endotoxin quickly and effectively, and when the LTP treatment time was increased, the concentrations of bacterial endotoxin decreased gradually (after 60 s plasma treatment, its inactivation effect was beyond the Chinese pharmacopoeia standard), and the average survival time of mice gradually extended. The possible inactivation mechanisms are proposed to be related to reactive oxygen species (ROSs).

On-site SiH4 generator using hydrogen plasma generated in slit-type narrow gap

NASA Astrophysics Data System (ADS)

Takei, Norihisa; Shinoda, Fumiya; Kakiuchi, Hiroaki; Yasutake, Kiyoshi; Ohmi, Hiromasa

2018-06-01

We have been developing an on-site silane (SiH4) generator based on use of the chemical etching reaction between solid silicon (Si) and the high-density H atoms that are generated in high-pressure H2 plasma. In this study, we have developed a slit-type plasma source for high-efficiency SiH4 generation. High-density H2 plasma was generated in a narrow slit-type discharge gap using a 2.45 GHz microwave power supply. The plasma’s optical emission intensity distribution along the slit was measured and the resulting distribution was reflected by both the electric power distribution and the hydrogen gas flow. Because the Si etching rate strongly affects the SiH4 generation rate, the Si etching behavior was investigated with respect to variations in the experimental parameters. The weight etch rate increased monotonically with increasing input microwave power. However, the weight etch rate decreased with increasing H2 pressure and an increasing plasma gap. This reduction in the etch rate appears to be related to shrinkage of the plasma generation area because increased input power is required to maintain a constant plasma area with increasing H2 pressure and the increasing plasma gap. Additionally, the weight etch rate also increases with increasing H2 flow rate. The SiH4 generation rate of the slit-type plasma source was also evaluated using gas-phase Fourier transform infrared absorption spectroscopy and the material utilization efficiencies of both Si and the H2 gas for SiH4 gas formation were discussed. The main etch product was determined to be SiH4 and the developed plasma source achieved a SiH4 generation rate of 10 sccm (standard cubic centimeters per minute) at an input power of 900 W. In addition, the Si utilization efficiency exceeded 60%.

Metal carbonyl vapor generation coupled with dielectric barrier discharge to avoid plasma quench for optical emission spectrometry.

PubMed

Cai, Yi; Li, Shao-Hua; Dou, Shuai; Yu, Yong-Liang; Wang, Jian-Hua

2015-01-20

The scope of dielectric barrier discharge (DBD) microplasma as a radiation source for optical emission spectrometry (OES) is extended by nickel carbonyl vapor generation. We proved that metal carbonyl completely avoids the extinguishing of plasma, and it is much more suitable for matching the DBD excitation and OES detection with respect to significant DBD quenching by concomitant hydrogen when hydride generation is used. A concentric quartz UV reactor allows sample solution to flow through the central channel wherein to efficiently receive the uniformly distributed UV irradiation in the confined cylindrical space between the concentric tubes, which facilitates effective carbonyl generation in a nickel solution. The carbonyl is transferred into the DBD excitation chamber by an argon stream for nickel excitation, and the characteristic emission of nickel at 232.0 nm is detected by a charge-coupled device (CCD) spectrometer. A 1.0 mL sample solution results in a linear range of 5-100 μg L(-1) along with a detection limit of 1.3 μg L(-1) and a precision of 2.4% RSD at 50 μg L(-1). The present DBD-OES system is validated by nickel in certified reference materials.

Temporal VUV Emission Characteristics Related to Generations and Losses of Metastable Atoms in Xenon Pulsed Barrier Discharge

NASA Astrophysics Data System (ADS)

Motomura, Hideki; Loo, Ka Hong; Ikeda, Yoshihisa; Jinno, Masafumi; Aono, Masaharu

Although xenon pulsed dielectric barrier discharge is one of the most promising substitutes for mercury low-pressure discharge for fluorescent lamps, the efficacy of xenon fluorescent lamp is not enough for practical use for general lighting. To improve the efficacy it is indispensable to clarify mechanisms of vacuum ultraviolet (VUV) emissions, which excite phosphor, from xenon discharge related to plasma characteristics. In this paper emission waveforms and temporal change of metastable atom density are measured and temporal VUV emission characteristics related to generations and losses of metastable atoms in xenon pulsed barrier discharge is investigated. It is shown that the lamp efficacy is improved by about 10% with shorter pulse in which the two VUV emission peaks in a pulse are overlapped. It is also shown that at the lower pressure of 1.3 kPa metastable atoms generated during on-period of the voltage pulse are not efficiently consumed for VUV emissions in the off-period of the voltage pulse because of lower rate of three-body collision and quenching. This fact is thought to be one of the reasons why the lamp efficacy is low at lower pressure.

Method of making a coating of a microtextured surface

DOEpatents

Affinito, John D [Tucson, AZ; Graff, Gordon L [West Richland, WA; Martin, Peter M [Kennewick, WA; Gross, Mark E [Pasco, WA; Burrows, Paul E [Kennewick, WA; Sapochak, Linda S [Henderson, NV

2004-11-02

A method for conformally coating a microtextured surface. The method includes flash evaporating a polymer precursor forming an evaporate, passing the evaporate to a glow discharge electrode creating a glow discharge polymer precursor plasma from the evaporate, cryocondensing the glow discharge polymer precursor plasma on the microtextured surface and crosslinking the glow discharge polymer precursor plasma thereon, wherein the crosslinking resulting from radicals created in the glow discharge polymer precursor plasma.

Control of the Helicity Content of a Gun-Generated Spheromak by Incorporating a Conducting Shell into a Magnetized Coaxial Plasma Gun

NASA Astrophysics Data System (ADS)

Matsumoto, Tadafumi; Sekiguchi, Jun'ichi; Asai, Tomohiko

In the formation of magnetized plasmoid by a magnetized coaxial plasma gun (MCPG), the magnetic helicity content of the generated plasmoid is one of the critical parameters. Typically, the bias coil to generate a poloidal flux is mounted either on the outer electrode or inside the inner electrode. However, most of the flux generated in the conventional method spreads even radially outside of the formation region. Thus, only a fraction of the total magnetic flux is actually exploited for helicity generation in the plasmoid. In the proposed system, the plasma gun incorporates a copper shell mounted on the outer electrode. By changing the rise time of the discharge bias coil current and the geometrical structure of the shell, the magnetic field structure and its time evolution can be controlled. The effect of the copper shell has been numerically simulated for the actual gun structure, and experimentally confirmed. This may increase the magnetic helicity content results, through increased poloidal magnetic field.