Dust Deposition Events on Mt. Elbrus, Caucasus Mountains in the 21st Century Reconstructed from the Shallow Firn and Ice Cores (Invited)

NASA Astrophysics Data System (ADS)

Shahgedanova, M.; Kutuzov, S.; Mikhalenko, V.; Ginot, P.; Lavrentiev, I.

2013-12-01

This paper presents and discusses a record of dust deposition events reconstructed from the shallow firn and ice cores extracted on the Western Plateau, Mt. Elbrus, Caucasus Mountains, Russia. A combination of SEVIRI imagery, HYSPLIT trajectory model, meteorological and atmospheric optical depth data were used to establish timing of deposition events and source regions of dust with very high temporal (hours) and spatial (c. 50-100 km) resolution. The source regions of the desert dust transported to Mt. Elbrus were primarily located in the Middle East, in particular in eastern Syria and in the Syrian Desert at the border between Saudi Arabia, Iraq and Jordan. Northern Sahara, the foothills of the Djebel Akhdar Mountains in eastern Libya and the border region between Libya and Algeria were other important sources of desert dust. Dust sources in the Sahara were natural (e.g. palaeolakes and alluvial deposits in the foothills) while in the Middle East, dust entrainment occurred from both natural (e.g. dry river beds) and anthropogenic (e.g. agricultural fields) sources. The overall majority of dust deposition events occurred between March and June and, less frequently, dust deposition events occurred in February and October. In all cases, dust deposition was associated with depressions causing strong surface wind and dust uplift in the source areas, transportation of dust to the Caucasus with a strong south-westerly flow from the Sahara or southerly flow from the Middle East, merging of the dust clouds with precipitation-bearing weather fronts and precipitation over the Caucasus region. The Saharan depressions were vigorous and associated with stronger daily wind speeds of 20-30 m/s at the 700 hPa level; depressions forming over the Middle East and the associated wind speeds were weaker at 12-15 m/s. The Saharan depressions were less frequent than those carrying dust from the Middle East but higher dust loads were associated with the Saharan depressions. A higher frequency of dust deposition events on Mt. Elbrus was registered in 2007-2010 due to the prolonged drought in the Middle East resulting in a more frequent activation of dust sources, including agricultural fields abandoned because of the draught.

Dust deposition in southern Nevada and California, 1984-1989: Relations to climate, source area, and source lithology

NASA Astrophysics Data System (ADS)

Reheis, Marith C.; Kihl, Rolf

1995-05-01

Dust samples collected annually for 5 years from 55 sites in southern Nevada and California provide the first regional source of information on modern rates of dust deposition, grain size, and mineralogical and chemical composition relative to climate and to type and lithology of dust source. The average silt and clay flux (rate of deposition) in southern Nevada and southeastern California ranges from 4.3 to 15.7 g/m2/yr, but in southwestern California the average silt and clay flux is as high as 30 g/m2/yr. The climatic factors that affect dust flux interact with each other and with the factors of source type (playas versus alluvium), source lithology, geographic area, and human disturbance. Average dust flux increases with mean annual temperature but is not correlated to decreases in mean annual precipitation because the regional winds bring dust to relatively wet areas. In contrast, annual dust flux mostly reflects changes in annual precipitation (relative drought) rather than temperature. Although playa and alluvial sources produce about the same amount of dust per unit area, the total volume of dust from the more extensive alluvial sources is much larger. In addition, playa and alluvial sources respond differently to annual changes in precipitation. Most playas produce dust that is richer in soluble salts and carbonate than that from alluvial sources (except carbonate-rich alluvium). Gypsum dust may be produced by the interaction of carbonate dust and anthropogenic or marine sulfates. The dust flux in an arid urbanizing area may be as much as twice that before disturbance but decreases when construction stops. The mineralogic and major-oxide composition of the dust samples indicates that sand and some silt is locally derived and deposited, whereas clay and some silt from different sources can be far-traveled. Dust deposited in the Transverse Ranges of California by the Santa Ana winds appears to be mainly derived from sources to the north and east.

Desert Dust and Health: A Central Asian Review and Steppe Case Study.

PubMed

Sternberg, Troy; Edwards, Mona

2017-11-03

In Asian deserts environmental and anthropomorphic dust is a significant health risk to rural populations. Natural sources in dry landscapes are exacerbated by human activities that increase the vulnerability to dust and dust-borne disease vectors. Today in Central and Inner Asian drylands, agriculture, mining, and rapid development contribute to dust generation and community exposure. Thorough review of limited dust investigation in the region implies but does not quantify health risks. Anthropogenic sources, such as the drying of the Aral Sea, highlight the shifting dust dynamics across the Central EurAsian steppe. In the Gobi Desert, our case study in Khanbogd, Mongolia addressed large-scale mining's potential dust risk to the health of the local population. Dust traps showed variable exposure to particulates among herder households and town residents; dust density distribution indicated that sources beyond the mine need to be considered when identifying particulate sources. Research suggests that atmospheric dust from multiple causes may enhance human particulate exposure. Greater awareness of dust in greater Central Asia reflects community concern about related health implications. Future human well-being in the region will require more thorough information on dust emissions in the changing environment.

Desert Dust and Health: A Central Asian Review and Steppe Case Study

PubMed Central

Sternberg, Troy; Edwards, Mona

2017-01-01

In Asian deserts environmental and anthropomorphic dust is a significant health risk to rural populations. Natural sources in dry landscapes are exacerbated by human activities that increase the vulnerability to dust and dust-borne disease vectors. Today in Central and Inner Asian drylands, agriculture, mining, and rapid development contribute to dust generation and community exposure. Thorough review of limited dust investigation in the region implies but does not quantify health risks. Anthropogenic sources, such as the drying of the Aral Sea, highlight the shifting dust dynamics across the Central EurAsian steppe. In the Gobi Desert, our case study in Khanbogd, Mongolia addressed large-scale mining’s potential dust risk to the health of the local population. Dust traps showed variable exposure to particulates among herder households and town residents; dust density distribution indicated that sources beyond the mine need to be considered when identifying particulate sources. Research suggests that atmospheric dust from multiple causes may enhance human particulate exposure. Greater awareness of dust in greater Central Asia reflects community concern about related health implications. Future human well-being in the region will require more thorough information on dust emissions in the changing environment. PMID:29099792

High Latitude Dust Sources, Transport Pathways and Impacts

NASA Astrophysics Data System (ADS)

Bullard, J. E.; Baddock, M. C.; Darlington, E.; Mockford, T.; Van-Soest, M.

2017-12-01

Estimates from field studies, remote sensing and modelling all suggest around 5% of global dust emissions originate in the high latitudes (≥50°N and ≥40°S), a similar proportion to that from the USA (excluding Alaska) or Australia. This paper identifies contemporary sources of dust within the high latitudes and their role within local, regional and hemispherical environmental systems. Field data and remote sensing analyses are used to identify the environmental and climatic conditions that characterize high latitude dust sources in both hemispheres. Examples from Arctic and sub-Arctic dust sources are used to demonstrate and explain the different regional relationships among dust emissions, glacio-fluvial dynamics and snow cover. The relative timing of dust input to high latitude terrestrial, cryospheric and marine systems determines its short to medium term environmental impact. This is highlighted through quantifying the importance of locally-redistributed dust as a nutrient input to high latitude soils and lakes in West Greenland.

Performance evaluation of CESM in simulating the dust cycle

NASA Astrophysics Data System (ADS)

Parajuli, S. P.; Yang, Z. L.; Kocurek, G.; Lawrence, D. M.

2014-12-01

Mineral dust in the atmosphere has implications for Earth's radiation budget, biogeochemical cycles, hydrological cycles, human health and visibility. Mineral dust is injected into the atmosphere during dust storms when the surface winds are sufficiently strong and the land surface conditions are favorable. Dust storms are very common in specific regions of the world including the Middle East and North Africa (MENA) region, which contains more than 50% of the global dust sources. In this work, we present simulation of the dust cycle under the framework of CESM1.2.2 and evaluate how well the model captures the spatio-temporal characteristics of dust sources, transport and deposition at global scale, especially in dust source regions. We conducted our simulations using two existing erodibility maps (geomorphic and topographic) and a new erodibility map, which is based on the correlation between observed wind and dust. We compare the simulated results with MODIS satellite data, MACC reanalysis data, and AERONET station data. Comparison with MODIS satellite data and MACC reanalysis data shows that all three erodibility maps generally reproduce the spatio-temporal characteristics of dust optical depth globally. However, comparison with AERONET station data shows that the simulated dust optical depth is generally overestimated for all erodibility maps. Results vary greatly by region and scale of observational data. Our results also show that the simulations forced by reanalysis meteorology capture the overall dust cycle more realistically compared to the simulations done using online meteorology.

Dust Storm over the Middle East: Retrieval Approach, Source Identification, and Trend Analysis

NASA Astrophysics Data System (ADS)

Moridnejad, A.; Karimi, N.; Ariya, P. A.

2014-12-01

The Middle East region has been considered to be responsible for approximately 25% of the Earth's global emissions of dust particles. By developing Middle East Dust Index (MEDI) and applying to 70 dust storms characterized on MODIS images and occurred during the period between 2001 and 2012, we herein present a new high resolution mapping of major atmospheric dust source points participating in this region. To assist environmental managers and decision maker in taking proper and prioritized measures, we then categorize identified sources in terms of intensity based on extracted indices for Deep Blue algorithm and also utilize frequency of occurrence approach to find the sensitive sources. In next step, by implementing the spectral mixture analysis on the Landsat TM images (1984 and 2012), a novel desertification map will be presented. The aim is to understand how human perturbations and land-use change have influenced the dust storm points in the region. Preliminary results of this study indicate for the first time that c.a., 39 % of all detected source points are located in this newly anthropogenically desertified area. A large number of low frequency sources are located within or close to the newly desertified areas. These severely desertified regions require immediate concern at a global scale. During next 6 months, further research will be performed to confirm these preliminary results.

Characterization of Asian Dust Properties Near Source Region During ACE-Asia

NASA Technical Reports Server (NTRS)

Tsay, Si-Chee; Hsu, N. Christina; King, Michael D.; Kaufman, Yoram J.; Herman, Jay R.

2004-01-01

Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian aerosols is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia campaign, we have acquired ground- based (temporal) and satellite (spatial) measurements to infer aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over this region. The inclusion of flux measurements permits the determination of aerosol radiative flux in addition to measurements of loading and optical depth. At the time of the Terra/MODIS, SeaWiFS, TOMS and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. In this paper, we will demonstrate new capability of the Deep Blue algorithm to track the evolution of the Asian dust storm from sources to sinks. Although there are large areas often covered by clouds in the dust season in East Asia, this algorithm is able to distinguish heavy dust from clouds over the entire regions. Examination of the retrieved daily maps of dust plumes over East Asia clearly identifies the sources contributing to the dust loading in the atmosphe. We have compared the satellite retrieved aerosol optical thickness to the ground-based measurements and obtained a reasonable agreement between these two. Our results also indicate that there is a large difference in the retrieved value of spectral single scattering albedo of windblown dust between different sources in East Asia.

Development of High-Resolution Dynamic Dust Source Function - A Case Study with a Strong Dust Storm in a Regional Model

NASA Technical Reports Server (NTRS)

Kim, Dongchul; Chin, Mian; Kemp, Eric M.; Tao, Zhining; Peters-Lidard, Christa D.; Ginoux, Paul

2017-01-01

A high-resolution dynamic dust source has been developed in the NASA Unified-Weather Research and Forecasting (NU-WRF) model to improve the existing coarse static dust source. In the new dust source map, topographic depression is in 1-km resolution and surface bareness is derived using the Normalized Difference Vegetation Index (NDVI) data from Moderate Resolution Imaging Spectroradiometer (MODIS). The new dust source better resolves the complex topographic distribution over the Western United States where its magnitude is higher than the existing, coarser resolution static source. A case study is conducted with an extreme dust storm that occurred in Phoenix, Arizona in 0203 UTC July 6, 2011. The NU-WRF model with the new high-resolution dynamic dust source is able to successfully capture the dust storm, which was not achieved with the old source identification. However the case study also reveals several challenges in reproducing the time evolution of the short-lived, extreme dust storm events.

Development of High-Resolution Dynamic Dust Source Function -A Case Study with a Strong Dust Storm in a Regional Model

PubMed Central

Kim, Dongchul; Chin, Mian; Kemp, Eric M.; Tao, Zhining; Peters-Lidard, Christa D.; Ginoux, Paul

2018-01-01

A high-resolution dynamic dust source has been developed in the NASA Unified-Weather Research and Forecasting (NU-WRF) model to improve the existing coarse static dust source. In the new dust source map, topographic depression is in 1-km resolution and surface bareness is derived using the Normalized Difference Vegetation Index (NDVI) data from Moderate Resolution Imaging Spectroradiometer (MODIS). The new dust source better resolves the complex topographic distribution over the Western United States where its magnitude is higher than the existing, coarser resolution static source. A case study is conducted with an extreme dust storm that occurred in Phoenix, Arizona in 02-03 UTC July 6, 2011. The NU-WRF model with the new high-resolution dynamic dust source is able to successfully capture the dust storm, which was not achieved with the old source identification. However the case study also reveals several challenges in reproducing the time evolution of the short-lived, extreme dust storm events. PMID:29632432

Development of High-Resolution Dynamic Dust Source Function -A Case Study with a Strong Dust Storm in a Regional Model.

PubMed

Kim, Dongchul; Chin, Mian; Kemp, Eric M; Tao, Zhining; Peters-Lidard, Christa D; Ginoux, Paul

2017-06-01

A high-resolution dynamic dust source has been developed in the NASA Unified-Weather Research and Forecasting (NU-WRF) model to improve the existing coarse static dust source. In the new dust source map, topographic depression is in 1-km resolution and surface bareness is derived using the Normalized Difference Vegetation Index (NDVI) data from Moderate Resolution Imaging Spectroradiometer (MODIS). The new dust source better resolves the complex topographic distribution over the Western United States where its magnitude is higher than the existing, coarser resolution static source. A case study is conducted with an extreme dust storm that occurred in Phoenix, Arizona in 02-03 UTC July 6, 2011. The NU-WRF model with the new high-resolution dynamic dust source is able to successfully capture the dust storm, which was not achieved with the old source identification. However the case study also reveals several challenges in reproducing the time evolution of the short-lived, extreme dust storm events.

Early-Holocene greening of the Afro-Asian dust belt changed sources of mineral dust in West Asia

NASA Astrophysics Data System (ADS)

Sharifi, Arash; Murphy, Lisa N.; Pourmand, Ali; Clement, Amy C.; Canuel, Elizabeth A.; Naderi Beni, Abdolmajid; Lahijani, Hamid A. K.; Delanghe, Doriane; Ahmady-Birgani, Hesam

2018-01-01

Production, transport and deposition of mineral dust have significant impacts on different components of the Earth systems through time and space. In modern times, dust plumes are associated with their source region(s) using satellite and land-based measurements and trajectory analysis of air masses through time. Reconstruction of past changes in the sources of mineral dust as related to changes in climate, however, must rely on the knowledge of the geochemical and mineralogical composition of modern and paleo-dust, and that of their potential source origins. In this contribution, we present a 13,000-yr record of variations in radiogenic Sr-Nd-Hf isotopes and Rare Earth Element (REE) anomalies as well as dust grain size from an ombrotrophic (rain fed) peat core in NW Iran as proxies of past changes in the sources of dust over the interior of West Asia. Our data shows that although the grain size of dust varies in a narrow range through the entire record, the geochemical fingerprint of dust particles deposited during the low-flux, early Holocene period (11,700-6,000 yr BP) is distinctly different from aerosols deposited during high dust flux periods of the Younger Dryas and the mid-late Holocene (6,000-present). Our findings indicate that the composition of mineral dust deposited at the study site changed as a function of prevailing atmospheric circulation regimes and land exposure throughout the last deglacial period and the Holocene. Simulations of atmospheric circulation over the region show the Northern Hemisphere Summer Westerly Jet was displaced poleward across the study area during the early Holocene when Northern Hemisphere insolation was higher due to the Earth's orbital configuration. This shift, coupled with lower dust emissions simulated based on greening of the Afro-Asian Dust Belt during the early Holocene likely led to potential sources in Central Asia dominating dust export to West Asia during this period. In contrast, the dominant western and southwest Asian and Eastern African sources have prevailed during the mid-Holocene to modern times.

Case study of dust event sources from the Gobi and Taklamakan deserts: An investigation of the horizontal evolution and topographical effect using numerical modeling and remote sensing.

PubMed

Fan, Jin; Yue, Xiaoying; Sun, Qinghua; Wang, Shigong

2017-06-01

A severe dust event occurred from April 23 to April 27, 2014, in East Asia. A state-of-the-art online atmospheric chemistry model, WRF/Chem, was combined with a dust model, GOCART, to better understand the entire process of this event. The natural color images and aerosol optical depth (AOD) over the dust source region are derived from datasets of moderate resolution imaging spectroradiometer (MODIS) loaded on a NASA Aqua satellite to trace the dust variation and to verify the model results. Several meteorological conditions, such as pressure, temperature, wind vectors and relative humidity, are used to analyze meteorological dynamic. The results suggest that the dust emission occurred only on April 23 and 24, although this event lasted for 5days. The Gobi Desert was the main source for this event, and the Taklamakan Desert played no important role. This study also suggested that the landform of the source region could remarkably interfere with a dust event. The Tarim Basin has a topographical effect as a "dust reservoir" and can store unsettled dust, which can be released again as a second source, making a dust event longer and heavier. Copyright © 2016. Published by Elsevier B.V.

Enhancing weak transient signals in SEVIRI false colour imagery: application to dust source detection in southern Africa

NASA Astrophysics Data System (ADS)

Murray, Jon E.; Brindley, Helen E.; Bryant, Robert G.; Russell, Jacqui E.; Jenkins, Katherine F.

2013-04-01

Understanding the processes governing the availability and entrainment of mineral dust into the atmosphere requires dust sources to be identified and the evolution of dust events to be monitored. To achieve this aim a wide range of approaches have been developed utilising observations from a variety of different satellite sensors. Global maps of source regions and their relative strengths have been derived from instruments in low Earth orbit (e.g. Total Ozone Monitoring Spectrometer (TOMS) (Prospero et al., 2002), MODerate resolution Imaging Spectrometer (MODIS) (Ginoux et al., 2012)). Instruments such as MODIS can also be used to improve precise source location (Baddock et al., 2009) but the information available is restricted to the satellite overpass times which may not be coincident with active dust emission from the source. Hence, at a regional scale, some of the more successful approaches used to characterise the activity of different sources use high temporal resolution data available from instruments in geostationary orbit. For example, the widely used red-green-blue (RGB) dust scheme developed by Lensky and Rosenfeld (2008) (hereafter LR2008) makes use of observations from selected thermal channels of the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) in a false colour rendering scheme in which dust appears pink. This scheme has provided the basis for numerous studies of north African dust sources and factors governing their activation (e.g. Schepanski et al., 2007, 2009, 2012). However, the LR2008 imagery can fail to identify dust events due to the effects of atmospheric moisture, variations in dust layer height and optical properties, and surface conditions (Brindley et al., 2012). Here we introduce a new method designed to circumvent some of these issues and enhance the signature of dust events using observations from SEVIRI. The approach involves the derivation of a composite clear-sky signal for selected channels on an individual time-step and pixel basis. These composite signals are subtracted from each observation in the relevant channels to enhance weak transient signals associated with low levels of dust emission. Different channel combinations are then rendered in false colour imagery to better identify dust source locations and activity. We have applied this new clear-sky difference (CSD) algorithm over three key source regions in southern Africa: the Makgadikgadi Basin, Etosha Pan, and the Namibian and western South African coast. Case studies indicate that advantages associated with the CSD approach include an improved ability to detect dust and distinguish multiple sources, the observation of source activation earlier in the diurnal cycle, and an improved ability to pinpoint dust source locations. These advantages are confirmed by a survey of four-years of data, comparing the results obtained using the CSD technique with those derived from LR2008 dust imagery. On average the new algorithm more than doubles the number of dust events identified, with the greatest improvement for the Makgadigkadi Basin and coastal regions. We anticipate exploiting this new activation record derived using the CSD approach to better understand the surface and meteorological conditions controlling dust uplift and subsequent atmospheric transport.

Detection of anthropogenic dust using CALIPSO lidar measurements

NASA Astrophysics Data System (ADS)

Huang, J. P.; Liu, J. J.; Chen, B.; Nasiri, S. L.

2015-10-01

Anthropogenic dusts are those produced by human activities on disturbed soils, which are mainly cropland, pastureland, and urbanized regions, and are a subset of the total dust load which includes natural sources from desert regions. Our knowledge of anthropogenic dusts is still very limited due to a lack of data. To understand the contribution of anthropogenic dust to the total global dust load, it is important to identify it apart from total dust. In this study, a new technique for distinguishing anthropogenic dust from natural dust is proposed by using Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) dust and planetary boundary layer (PBL) height retrievals along with a land use data set. Using this technique, the global distribution of dust is analyzed and the relative contribution of anthropogenic and natural dust sources to regional and global emissions are estimated. Results reveal that local anthropogenic dust aerosol due to human activity, such as agriculture, industrial activity, transportation, and overgrazing, accounts for about 25 % of the global continental dust load. Of these anthropogenic dust aerosols, more than 53 % come from semi-arid and semi-wet regions. Annual mean anthropogenic dust column burden (DCB) values range from 0.42 g m-2, with a maximum in India, to 0.12 g m-2, with a minimum in North America. A better understanding of anthropogenic dust emission will enable us to focus on human activities in these critical regions and with such knowledge we will be more able to improve global dust models and to explore the effects of anthropogenic emission on radiative forcing, climate change, and air quality in the future.

Chemistry and Photochemistry at the Surface of Urban Road Dust and Photoactive Minerals

NASA Astrophysics Data System (ADS)

Styler, S. A.; Abou-Ghanem, M.; Wickware, B.

2017-12-01

Each year, over a billion tons of dust are released into the atmosphere from arid regions. After its emission, dust can undergo efficient long-range transport to urban centres, where it can interact with local pollution sources. Another source of dust in urban regions is road dust resuspension, which is the largest anthropogenic source of primary particulate matter in both Canada and the United States. Since dust contains light-absorbing components, including iron- and titanium-containing minerals, dust-catalyzed photochemical processes have the potential to influence both the lifetime of pollutants present at the dust surface and the composition of the surrounding atmosphere. To date, most studies of dust photochemistry have focused on TiO2-mediated processes, and no studies have explored trace gas uptake at the surface of road dust. Here, we present first results from aerosol and coated-wall flow tube investigations of ozone uptake at the surface of a suite of titanium-containing minerals and road dust collected in Edmonton, Alberta. Together, this work represents a significant advance in our understanding of chemistry and photochemistry at realistic environmental interfaces.

Properties of transported African mineral dust aerosols in the Mediterranean region

NASA Astrophysics Data System (ADS)

Denjean, Cyrielle; Chevaillier, Servanne; Gaimoz, Cécile; Grand, Noel; Triquet, Sylvain; Zapf, Pascal; Loisil, Rodrigue; Bourrianne, Thierry; Freney, Evelyn; Dupuy, Regis; Sellegri, Karine; Schwarzenbock, Alfons; Torres, Benjamin; Mallet, Marc; Cassola, Federico; Prati, Paolo; Formenti, Paola

2015-04-01

The transport of mineral dust aerosols is a global phenomenon with strong climate implications. Depending on the travel distance over source regions, the atmospheric conditions and the residence time in the atmosphere, various transformation processes (size-selective sedimentation, mixing, condensation of gaseous species, and weathering) can modify the physical and chemical properties of mineral dust, which, in turn, can change the dust's optical properties. The model predictions of the radiative effect by mineral dust still suffer of the lack of certainty of these properties, and their temporal evolution with transport time. Within the frame of the ChArMex project (Chemistry-Aerosol Mediterranean experiment, http://charmex.lsce.ipsl.fr/), one intensive airborne campaign (ADRIMED, Aerosol Direct Radiative Impact in the regional climate in the MEDiterranean region, 06 June - 08 July 2013) has been performed over the Central and Western Mediterranean, one of the two major transport pathways of African mineral dust. In this study we have set up a systematic strategy to determine the optical, physical and optical properties of mineral dust to be compared to an equivalent dataset for dust close to source regions in Africa. This study is based on airborne observations onboard the SAFIRE ATR-42 aircraft, equipped with state of the art in situ instrumentation to measure the particle scattering and backscattering coefficients (nephelometer at 450, 550, and 700 nm), the absorption coefficient (PSAP at 467, 530, and 660 nm), the extinction coefficient (CAPS at 530 nm), the aerosol optical depth (PLASMA at 340 to 1640 nm), the size distribution in the extended range 40 nm - 30 µm by the combination of different particle counters (SMPS, USHAS, FSSP, GRIMM) and the chemical composition obtained by filter sampling. The chemistry and transport model CHIMERE-Dust have been used to classify the air masses according to the dust origin and transport. Case studies of dust transport from known but differing origins (source regions in Tunisia, Algeria, and Mauritania) and at different times after transport, will be presented. Results will be compared to equivalent measurements over source regions interpreted in terms of the evolution of the particle size distribution, chemical composition and optical properties.

The southern Kalahari as a dust source: preliminary results from the field

USDA-ARS?s Scientific Manuscript database

The Kalahari encompasses one of the largest drylands in the Southern Hemisphere and it is a potentially large source of atmospheric dust in its relatively low-dust region. The severe iron depletion in the southern Indian and Atlantic Oceans, the ocean basins that receive much of the Kalahari dust, ...

Urban dust in the Guanzhong Basin of China, part I: A regional distribution of dust sources retrieved using satellite data.

PubMed

Long, Xin; Li, Nan; Tie, Xuexi; Cao, Junji; Zhao, Shuyu; Huang, Rujin; Zhao, Mudan; Li, Guohui; Feng, Tian

2016-01-15

Urban dust pollution has been becoming an outstanding environmental problem due to rapid urbanization in China. However, it is very difficult to construct an urban dust inventory, owing to its small horizontal scale and strong temporal/spatial variability. With the analysis of visual interpretation, maximum likelihood classification, extrapolation and spatial overlaying, we quantified dust source distributions of urban constructions, barrens and croplands in the Guanzhong Basin using various satellite data, including VHR (0.5m), Lansat-8 OLI (30 m) and MCD12Q1 (500 m). The croplands were the dominant dust sources, accounting for 40% (17,913 km(2)) of the study area in summer and 36% (17,913 km(2)) in winter, followed by barrens, accounting for 5% in summer and 10% in winter. Moreover, the total constructions were 126 km(2), including 84% of active and 16% inactive. In addition, 59% of the constructions aggregated on the only megacity of the study area, Xi'an. With high accuracy exceeding 88%, the proposed satellite-data based method is feasible and valuable to quantify distributions of dust sources. This study provides a new perspective to evaluate regional urban dust, which is seldom quantified and reported. In a companied paper (Part-2 of the study), the detailed distribution of the urban dust sources is applied in a dynamical/aerosol model (WRF-Dust) to assess the effect of dust sources on aerosol pollution. Copyright © 2015 Elsevier B.V. All rights reserved.

Dust sources and atmospheric circulation in concert controlling Saharan dust emission and transport towards the Western Mediterranean Basin

NASA Astrophysics Data System (ADS)

Schepanski, Kerstin; Mallet, Marc; Heinold, Bernd; Ulrich, Max

2017-04-01

Dust transported from north African source regions towards Europe is a ubiquitous phenomenon in the Mediterranean region, a geographic region that is in part densely populated. Besides its impacts on the atmospheric radiation budget, dust suspended in the atmosphere results in reduced air quality, which is generally sensed as a reduction in quality of life. Furthermore, the exposure to dust aerosols enhances the prevalence of respiratory diseases, which reduces the general human wellbeing, and ultimately results in an increased loss of working hours due to illness and hospitalization rates. Characteristics of the atmospheric dust life cycle that determine dust transport will be presented with focus on the ChArMEx special observation period in June and July 2013 using the atmosphere-dust model COSMO-MUSCAT (COSMO: Consortium for Small-scale MOdeling; MUSCAT: MUltiScale Chemistry Aerosol Transport Model). Modes of atmospheric circulation were identified from empirical orthogonal function (EOF) analysis of the geopotential height at 850 hPa for summer 2013 and compared to EOFs calculated from 1979-2015 ERA-Interim reanalysis. Generally, two different phases were identified. They are related to the eastward propagation of the subtropical ridge into the Mediterranean basin, the position of the Saharan heat low, and the predominant Iberian heat low. The relation of these centres of action illustrates a dipole pattern for enhanced (reduced) dust emission fluxes, stronger (weaker) meridional dust transport, and consequent increase (decrease) atmospheric dust concentrations and deposition fluxes. In concert, the results from this study aim at illustrating the relevance of knowing the dust source locations in concert with the atmospheric circulation. Ultimately, this study addresses the question of what is finally transported towards the Mediterranean basin and Europe from which source regions - and fostered by which atmospheric circulation pattern. Outcomes from this study contribute to the understanding of varying atmospheric mineral dust contributions to the aerosol burden affecting populated areas around Europe.

Using thermal infrared (TIR) data to characterize dust sources, dust fall and the linkage to climate in the Middle East

NASA Astrophysics Data System (ADS)

Mohammad, R.; Ramsey, M.; Scheidt, S. P.

2010-12-01

Prior to mineral dust deposition affecting albedo, aerosols can have direct and indirect effects on local to regional scale climate by changing both the shortwave and longwave radiative forcing. In addition, mineral dust causes health hazards, such as respiratory-related illnesses and deaths, loss of agricultural soil, and safety hazards to aviation and motorists due to reduced visibility. Previous work utilized satellite and ground-based TIR data to describe the direct longwave radiative effect of the Saharan Air Layer (SAL) over the Atlantic Ocean originating from dust storms in the Western Sahara. TIR emission spectroscopy was used to identify the spectral absorption features of that dust. The current research focuses on Kuwait and utilizes a comprehensive set of spatial, analytical and geological tools to characterize dust emissions and its radiative effects. Surface mineral composition maps for the Kuwait region were created using ASTER images and GIS datasets in order to identify the possible sources of wind-blown dust. Backward trajectory analysis using the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model suggests the dust source areas were located in Iraq, Syria, Jordan and Saudi Arabia. Samples collected from two dust storms (May and July 2010) were analyzed for their mineral composition and to validate the dust source areas identified by the modeling and remote sensing analysis. These air fall dust samples were collected in glass containers on a 13 meter high rooftop in the suburb of Rumaithiya in Kuwait. Additional samples will be collected to expand the analysis and their chemical compositions will be characterized by a combination of laboratory X-ray fluorescence (XRF), Scanning Electron Microscopy (SEM) and TIR emission spectroscopy. The overarching objective of this ongoing research is to both characterize the effects of mineral dust on climate as well as establish a predictive tool that can identify dust storm sources and potentially aid in establishing a more accurate prediction and warning system in the Middle East region.

Atmospheric dust events in Central Asia: Relationship to wind, soil type, and land use

USDA-ARS?s Scientific Manuscript database

Xinjiang Province is one of the most important source regions of atmospheric dust in China. Spatial-temporal characteristics of dust events in the region were investigated by time series analysis of annual dust event frequency and meteorological data collected at 101 stations in Xinjiang Province fr...

Atmospheric Movement of Microorganisms in Clouds of Desert Dust and Implications for Human Health

PubMed Central

Griffin, Dale W.

2007-01-01

Billions of tons of desert dust move through the atmosphere each year. The primary source regions, which include the Sahara and Sahel regions of North Africa and the Gobi and Takla Makan regions of Asia, are capable of dispersing significant quantities of desert dust across the traditionally viewed oceanic barriers. While a considerable amount of research by scientists has addressed atmospheric pathways and aerosol chemistry, very few studies to determine the numbers and types of microorganisms transported within these desert dust clouds and the roles that they may play in human health have been conducted. This review is a summary of the current state of knowledge of desert dust microbiology and the health impact that desert dust and its microbial constituents may have in downwind environments both close to and far from their sources. PMID:17630335

Atmospheric movement of microorganisms in clouds of desert dust and implications for human health

USGS Publications Warehouse

Griffin, Dale W.

2007-01-01

Billions of tons of desert dust move through the atmosphere each year. The primary source regions, which include the Sahara and Sahel regions of North Africa and the Gobi and Takla Makan regions of Asia, are capable of dispersing significant quantities of desert dust across the traditionally viewed oceanic barriers. While a considerable amount of research by scientists has addressed atmospheric pathways and aerosol chemistry, very few studies to determine the numbers and types of microorganisms transported within these desert dust clouds and the roles that they may play in human health have been conducted. This review is a summary of the current state of knowledge of desert dust microbiology and the health impact that desert dust and its microbial constituents may have in downwind environments both close to and far from their sources.

Atmospheric movement of microorganisms in clouds of desert dust and implications for human health.

PubMed

Griffin, Dale W

2007-07-01

Billions of tons of desert dust move through the atmosphere each year. The primary source regions, which include the Sahara and Sahel regions of North Africa and the Gobi and Takla Makan regions of Asia, are capable of dispersing significant quantities of desert dust across the traditionally viewed oceanic barriers. While a considerable amount of research by scientists has addressed atmospheric pathways and aerosol chemistry, very few studies to determine the numbers and types of microorganisms transported within these desert dust clouds and the roles that they may play in human health have been conducted. This review is a summary of the current state of knowledge of desert dust microbiology and the health impact that desert dust and its microbial constituents may have in downwind environments both close to and far from their sources.

Global dust sources detection using MODIS Deep Blue Collection 6 aerosol products

NASA Astrophysics Data System (ADS)

Pérez García-Pando, C.; Ginoux, P. A.

2015-12-01

Our understanding of the global dust cycle is limited by a dearth of information about dust sources, especially small-scale features which could account for a large fraction of global emissions. Remote sensing sensors are the most useful tool to locate dust sources. These sensors include microwaves, visible channels, and lidar. On the global scale, major dust source regions have been identified using polar orbiting satellite instruments. The MODIS Deep Blue algorithm has been particularly useful to detect small-scale sources such as floodplains, alluvial fans, rivers, and wadis , as well as to identify anthropogenic sources from agriculture. The recent release of Collection 6 MODIS aerosol products allows to extend dust source detection to the entire land surfaces, which is quite useful to identify mid to high latitude dust sources and detect not only dust from agriculture but fugitive dust from transport and industrial activities. This presentation will overview the advantages and drawbacks of using MODIS Deep Blue for dust detection, compare to other instruments (polar orbiting and geostationary). The results of Collection 6 with a new dust screening will be compared against AERONET. Applications to long range transport of anthropogenic dust will be presented.

Spatiotemporal Modelling of Dust Storm Sources Emission in West Asia

NASA Astrophysics Data System (ADS)

Khodabandehloo, E.; Alimohamdadi, A.; Sadeghi-Niaraki, A.; Darvishi Boloorani, A.; Alesheikh, A. A.

2013-09-01

Dust aerosol is the largest contributor to aerosol mass concentrations in the troposphere and has considerable effects on the air quality of spatial and temporal scales. Arid and semi-arid areas of the West Asia are one of the most important regional dust sources in the world. These phenomena directly or indirectly affecting almost all aspects life in almost 15 countries in the region. So an accurate estimate of dust emissions is very crucial for making a common understanding and knowledge of the problem. Because of the spatial and temporal limits of the ground-based observations, remote sensing methods have been found to be more efficient and useful for studying the West Asia dust source. The vegetation cover limits dust emission by decelerating the surface wind velocities and therefore reducing the momentum transport. While all models explicitly take into account the change of wind speed and soil moisture in calculating dust emissions, they commonly employ a "climatological" land cover data for identifying dust source locations and neglect the time variation of surface bareness. In order to compile the aforementioned model, land surface features such as soil moisture, texture, type, and vegetation and also wind speed as atmospheric parameter are used. Having used NDVI data show significant change in dust emission, The modeled dust emission with static source function in June 2008 is 17.02 % higher than static source function and similar result for Mach 2007 show the static source function is 8.91 % higher than static source function. we witness a significant improvement in accuracy of dust forecasts during the months of most soil vegetation changes (spring and winter) compared to outputs resulted from static model, in which NDVI data are neglected.

Alpine lakes preserve mineral dust signatures: Implications for long-range mineral dust transport and Last Glacial Maximum (LGM) tornado frequency in the United States

NASA Astrophysics Data System (ADS)

Bhattacharya, A.; Lora, J. M.; Pollen, A.; Vollmer, T.; Thomas, M.; Leithold, E. L.; Mitchell, J.; Tripati, A.

2016-12-01

The net amount of mineral dust accumulation in arid and semi-arid regions might not be entirely sourced locally or even regionally; in fact, new evidence suggests that there could be significant contributions from distal sources. The contribution from the distal sources needs to be identified, and accounted for, in order to accurately understand the meteorological and climatologic factors, both regional and global, that control mineral dust accumulation in arid and semi-arid regions. Most importantly, if identified, the two components of mineral dust accumulation- fine fraction (typically <4 microns) and coarse fraction (typically >25 microns)- could provide critical information about regional as well as global climate. There are large-scale climatological controls on the finer fraction of mineral dust, while the coarser fraction is related to intense invents (i.e., the occurrence of cyclones). However, studies attempting to separate these two size fractions in terrestrial archives have been limited. Here we separate the two size fractions using grain size analysis, and use trace element analysis in each size fraction to identify contributing source regions. We apply this technique to well-dated cores collected from three lakes that are distributed across the western, southwestern and Great Plains in the United States: Pear Lake in the Sierra Nevada Mountains (CA), Senator Beck Lake in the San Juan Mountains (CO), and North Lake (WY). These lakes are uniquely situated to monitor dust fluxes; previous studies have demonstrated that sedimentation in these lakes are dominated by mineral dust accumulation; there is also evidence of remotely and locally sourced dust in these lakes, and of textural differences between the two types of dust fractions. We compare our results with previously published data on dust from loess deposits in the United States, and isotopic modeling (LMDZ). We find evidence that the finer-grain size fraction in alpine lake cores could be of remote origin; work is underway to quantify this contribution. Most importantly, we find that during the Last Glacial Maximum (LGM) the Great Plains may not have witnessed an increase in the incidence of tornado frequency. Acknowledgements: James Sigman, Jacob Ashford, Jason Neff and Amato Evan

Numerical simulations of Asian dust storms using a coupled climate-aerosol microphysical model

NASA Astrophysics Data System (ADS)

Su, Lin; Toon, Owen B.

2009-07-01

We have developed a three-dimensional coupled microphysical/climate model based on the National Center for Atmospheric Research Community Atmospheres Model and the University of Colorado/NASA Community Aerosol and Radiation Model for Atmospheres. We have used the model to investigate the sources, removal processes, transport, and optical properties of Asian dust aerosol and its impact on downwind regions. The model simulations are conducted primarily during the time frame of the Aerosol Characterization Experiment-Asia field experiment (March-May 2001) since considerable in situ data are available at that time. Our dust source function follows Ginoux et al. (2001). We modified the dust source function by using the friction velocity instead of the 10-m wind based on wind erosion theory, by adding a size-dependent threshold friction velocity following Marticorena and Bergametti (1995) and by adding a soil moisture correction. A Weibull distribution is implemented to estimate the subgrid-scale wind speed variability. We use eight size bins for mineral dust ranging from 0.1 to 10 μm radius. Generally, the model reproduced the aerosol optical depth retrieved by the ground-based Aerosol Robotic Network (AERONET) Sun photometers at six study sites ranging in location from near the Asian dust sources to the Eastern Pacific region. By constraining the dust complex refractive index from AERONET retrievals near the dust source, we also find the single-scattering albedo to be consistent with AERONET retrievals. However, large regional variations are observed due to local pollution. The timing of dust events is comparable to the National Institute for Environmental Studies (NIES) lidar data in Beijing and Nagasaki. However, the simulated dust aerosols are at higher altitudes than those observed by the NIES lidar.

The effect of radiation pressure on spatial distribution of dust inside H II regions

NASA Astrophysics Data System (ADS)

Ishiki, Shohei; Okamoto, Takashi; Inoue, Akio K.

2018-02-01

We investigate the impact of radiation pressure on spatial dust distribution inside H II regions using one-dimensional radiation hydrodynamic simulations, which include absorption and re-emission of photons by dust. In order to investigate grain-size effects as well, we introduce two additional fluid components describing large and small dust grains in the simulations. Relative velocity between dust and gas strongly depends on the drag force. We include collisional drag force and coulomb drag force. We find that, in a compact H II region, a dust cavity region is formed by radiation pressure. Resulting dust cavity sizes (˜0.2 pc) agree with observational estimates reasonably well. Since dust inside an H II region is strongly charged, relative velocity between dust and gas is mainly determined by the coulomb drag force. Strength of the coulomb drag force is about 2 order of magnitude larger than that of the collisional drag force. In addition, in a cloud of mass 105 M⊙, we find that the radiation pressure changes the grain-size distribution inside H II regions. Since large (0.1 μm) dust grains are accelerated more efficiently than small (0.01 μm) grains, the large-to-small grain mass ratio becomes smaller by an order of magnitude compared with the initial one. Resulting dust-size distributions depend on the luminosity of the radiation source. The large and small grain segregation becomes weaker when we assume stronger radiation source, since dust grain charges become larger under stronger radiation and hence coulomb drag force becomes stronger.

Sr-Nd-Hf isotopic fingerprinting of transatlantic dust derived from North Africa

NASA Astrophysics Data System (ADS)

Zhao, Wancang; Balsam, William; Williams, Earle; Long, Xiaoyong; Ji, Junfeng

2018-03-01

Long-range transport of African dust plays an important role in understanding dust-climate relationships including dust source areas, dust pathways and associated atmospheric and/or oceanic processes. Clay-sized Sr-Nd-Hf isotopic compositions can be used as geochemical fingerprints to constrain dust provenance and the pathways of long-range transported mineral dust. We investigated the clay-sized Sr-Nd-Hf isotopic composition of surface samples along four transects bordering the Sahara Desert. The transects are from Mali, Niger/Benin/Togo, Egypt and Morocco. Our results show that the Mali transect on the West African Craton (WAC) produces lower εNd (εNd-mean = -16.38) and εHf (εHf-mean = -9.59) values than the other three transects. The Egyptian transect exhibits the lowest 87Sr/86Sr ratios (87Sr/86Srmean = 0.709842), the highest εHf (εHf-mean = -0.34) and εNd values of the four transects. Comparison of the clay-sized Sr-Nd-Hf isotopic values from our North African samples to transatlantic African dust collected in Barbados demonstrates that the dust's provenance is primarily the western Sahel and Sahara as well as the central Sahel. Summer emission dust is derived mainly from the western Sahel and Sahara regions. The source of transatlantic dust in spring and autumn is more varied than in the summer and includes dust not only from western areas, but also south central areas. Comparison of the Sr-Nd-Hf isotopic fingerprints between the source and sink of transatlantic dust also suggests that a northwestward shift in dust source occurs from the winter, through the spring and into the summer. The isotopic data we develop here provide another tool for discriminating changes in dust archives resulting from paleoenvironmental evolution of source regions.

Regional and climatic controls on seasonal dust deposition in the southwestern U.S.

USGS Publications Warehouse

Reheis, M.C.; Urban, F.E.

2011-01-01

Vertical dust deposition rates (dust flux) are a complex response to the interaction of seasonal precipitation, wind, changes in plant cover and land use, dust source type, and local vs. distant dust emission in the southwestern U.S. Seasonal dust flux in the Mojave-southern Great Basin (MSGB) deserts, measured from 1999 to 2008, is similar in summer-fall and winter-spring, and antecedent precipitation tends to suppress dust flux in winter-spring. In contrast, dust flux in the eastern Colorado Plateau (ECP) region is much larger in summer-fall than in winter-spring, and twice as large as in the MSGB. ECP dust is related to wind speed, and in the winter-spring to antecedent moisture. Higher summer dust flux in the ECP is likely due to gustier winds and runoff during monsoonal storms when temperature is also higher. Source types in the MSGB and land use in the ECP have important effects on seasonal dust flux. In the MSGB, wet playas produce salt-rich dust during wetter seasons, whereas antecedent and current moisture suppress dust emission from alluvial and dry-playa sources during winter-spring. In the ECP under drought conditions, dust flux at a grazed-and-plowed site increased greatly, and also increased at three annualized, previously grazed sites. Dust fluxes remained relatively consistent at ungrazed and currently grazed sites that have maintained perennial vegetation cover. Under predicted scenarios of future climate change, these results suggest that an increase in summer storms may increase dust flux in both areas, but resultant effects will depend on source type, land use, and vegetation cover. ?? 2011.

A parameterization of dust emission (PM10) fluxes of dust events observed at Naiman in Inner Mongolia using the monitored tower data

NASA Astrophysics Data System (ADS)

Park, Soon-Ung; Ju, Jae-Won; Lee, In-Hye; Joo, Seung Jin

2016-09-01

The optimal regression equations for the dust emission flux parameterized with the friction velocity (u*) only, the friction velocity with the threshold friction velocity (u*t) and the friction velocity together with the flux Richardson number (Rf) in the dust source region are derived using the sonic anemometer measured momentum and kinematic heat fluxes at 8 m height and the two-level (3 m and 15 m height) measured PM10 concentrations from a 20-m monitoring tower located at Naiman in the Asian dust source region in China for the period from March 2013 to November 2014. The analysis period is divided into three sub-periods based on the Normalized Difference Vegetation Index (NDVI) to eliminate the effect of vegetation on the dust emission flux. The dust event is identified as a peak half hourly mean dust concentration (PM10) at 3 m height exceeding the sub-period mean dust concentration plus one standard deviation of the sub-period. The total of 317 dust events is identified with the highest number of dust event of 18.8 times a month in summer. The optimal regression equations of the dust emission flux (Fc) for dust events parameterized with u* and Rf are found to simulate quite well the dust emission flux estimated by the observed data at the site for all periods especially for the unstable stratification, suggesting the potential usefulness of these equations parameterized by u* with Rf rather than those by u* only and u* together with u*t for the estimation of the dust emission flux in the Asian dust source region.

Optical, physical and chemical properties of transported African mineral dust aerosols in the Mediterranean region

NASA Astrophysics Data System (ADS)

Denjean, Cyrielle; Di Biagio, Claudia; Chevaillier, Servanne; Gaimoz, Cécile; Grand, Noel; Loisil, Rodrigue; Triquet, Sylvain; Zapf, Pascal; Roberts, Greg; Bourrianne, Thierry; Torres, Benjamin; Blarel, Luc; Sellegri, Karine; Freney, Evelyn; Schwarzenbock, Alfons; Ravetta, François; Laurent, Benoit; Mallet, Marc; Formenti, Paola

2014-05-01

The transport of mineral dust aerosols is a global phenomenon with strong climate implications. Depending on the travel distance over source regions, the atmospheric conditions and the residence time in the atmosphere, various transformation processes (size-selective sedimentation, mixing, condensation of gaseous species, and weathering) can modify the physical and chemical properties of mineral dust, which, in turn, can change the dust's optical properties. The model predictions of the radiative effect by mineral dust still suffer of the lack of certainty of these properties, and their temporal evolution with transport time. Within the frame of the ChArMex project (Chemistry-Aerosol Mediterranean experiment, http://charmex.lsce.ipsl.fr/), two intensive airborne campaigns (TRAQA, TRansport and Air QuAlity, 18 June - 11 July 2012, and ADRIMED, Aerosol Direct Radiative Impact in the regional climate in the MEDiterranean region, 06 June - 08 July 2013) have been performed over the Central and Western Mediterranean, one of the two major transport pathways of African mineral dust. In this study we have set up a systematic strategy to determine the optical, physical and optical properties of mineral dust to be compared to an equivalent dataset for dust close to source regions in Africa. This study is based on airborne observations onboard the SAFIRE ATR-42 aircraft, equipped with state of the art in situ instrumentation to measure the particle scattering and backscattering coefficients (nephelometer at 450, 550, and 700 nm), the absorption coefficient (PSAP at 467, 530, and 660 nm), the extinction coefficient (CAPS at 530 nm), the aerosol optical depth (PLASMA at 340 to 1640 nm), the size distribution in the extended range 40 nm - 30 µm by the combination of different particle counters (SMPS, USHAS, FSSP, GRIMM) and the chemical composition obtained by filter sampling. The chemistry and transport model CHIMERE-Dust have been used to classify the air masses according to the dust origin and transport. Case studies of dust transport from known but differing origins (source regions in Tunisia, Algeria, and Mauritania) and at different times after transport, will be presented. Results will be compared to equivalent measurements over source regions interpreted in terms of the evolution of the particle size distribution, chemical composition and optical properties.

Linking Barbados Mineral Dust Aerosols to North African Sources Using Elemental Composition and Radiogenic Sr, Nd, and Pb Isotope Signatures

NASA Astrophysics Data System (ADS)

Bozlaker, Ayse; Prospero, Joseph M.; Price, Jim; Chellam, Shankararaman

2018-01-01

Large quantities of African dust are carried across the Atlantic to the Caribbean Basin and southern United States where it plays an important role in the biogeochemistry of soils and waters and in air quality. Dusts' elemental and isotopic composition was comprehensively characterized in Barbados during the summers of 2013 and 2014, the season of maximum dust transport. Although total suspended insoluble particulate matter (TSIP) mass concentrations varied significantly daily and between the two summers, the abundances (μg element/g TSIP) of 50 elements during "high-dust days" (HDD) were similar. Aerosols were regularly enriched in Na, Cu, Zn, As, Se, Mo, Cd, Sn, Sb, and W relative to the upper continental crust. Enrichment of these elements, many of which are anthropogenically emitted, was significantly reduced during HDD, attributed to mixing and dilution with desert dust over source regions. Generally, Ti/Al, Si/Al, Ca/Al, Ti/Fe, Si/Fe, and Ca/Fe ratios during HDD differed from their respective values in hypothesized North African source regions. Nd isotope composition was relatively invariant for "low-dust days" (LDD) and HDD. In contrast, HDD-aerosols were more radiogenic exhibiting higher 87Sr/86Sr, 206Pb/204Pb, 207Pb/204Pb, and 208Pb/204Pb ratios compared to LDD. Generally, Barbados aerosols' composition ranged within narrow limits and was much more homogeneous than that of hypothesized African source soils. Our results suggest that summertime Barbados aerosols are dominated by a mixture of particles originating from sources in the Sahara-Sahel regions. The Bodélé Depression, long suspected as a major source, appears to be an insignificant contributor of summertime western Atlantic dust.

The Dynamics and Characteristics of Aeolian Dust in Dryland Central Asia: Possible Impacts on Respiratory Health in the Aral Sea Basin

NASA Astrophysics Data System (ADS)

Wiggs, G. F.; O'Hara, S.; Wegerdt, J.; van der Meer, J.; Small, I.; Hubbard, R.

2003-12-01

Over the last 40 years over 36,000 km2 of the former Aral Sea bed have been exposed creating a potentially significant aeolian dust source. It is widely believed, but little researched, that increased dust storm activity in the region has had a major impact on human health. In this paper we report the findings of a study into the link between dust exposure and respiratory health amongst children in the Autonomous Republic of Karakalpakstan, located on the southern shore of the Aral Sea. Data were collected over a 12 month period at 16 sites located within a broad transect running north to south through Karakalpakstan. At each site monthly measurements of dust deposition were undertaken linked with daily meteorological data at 6 stations. At 3 sites weekly measurements of PM10 were also carried out. Approximately 100 children (aged 7-10 years) were randomly selected within 5 km of each dust trap site and data were collected on their respiratory health and environmental exposures. Lung function data were also collected using a handheld spirometer. A linear regression model was used to predict lung function for the children incorporating variables for Forced Expiratory Volume in one second (FEV1), age, gender, height and weight and we estimated the impact of dust deposition rates on the odds of having abnormal lung function using logistic regression. The findings indicate that dust deposition rates across the region are high with sites located near the former shore of the sea being the worst affected. For these northerly regions the former Aral Sea bed is the most likely source of dust. The situation for the rest of the country seems to be far more complex. In these regions it appears that local sources (agricultural fields, abandoned irrigation grounds, overgrazed dunes, and unpaved roads) and more distant sources to the south and south-west represent significant sediment providers, particularly in the early summer when agricultural fields are ploughed. We found some evidence of a dose-related impact of dust levels on lung function. These associations were statistically significant for all measures of dust exposure but were most marked for levels of winter dust exposure and level of PM2.5 exposure. The results from this study suggest that aeolian dust dynamics in the region are spatially and temporally highly variable and, counter to local and regional perceptions, the former bed of the Aral Sea does not appear to be the only significant source. Nevertheless, there is also evidence of a dose-related impact of airborne dust on the risk of having abnormally low lung function in children living in the Aral Sea Area.

Improving the simulation of convective dust storms in regional-to-global models

EPA Science Inventory

Convective dust storms have significant impacts on atmospheric conditions and air quality and are a major source of dust uplift in summertime. However, regional-to-global models generally do not accurately simulate these storms, a limitation that can be attributed to (1) using a ...

Emerging ecological datasets with application for modeling North American dust emissions

NASA Astrophysics Data System (ADS)

McCord, S.; Stauffer, N. G.; Garman, S.; Webb, N.

2017-12-01

In 2011 the US Bureau of Land Management (BLM) established the Assessment, Inventory and Monitoring (AIM) program to monitor the condition of BLM land and to provide data to support evidence-based management of multi-use public lands. The monitoring program shares core data collection methods with the Natural Resources Conservation Service's (NRCS) National Resources Inventory (NRI), implemented on private lands nationally. Combined, the two programs have sampled >30,000 locations since 2003 to provide vegetation composition, vegetation canopy height, the size distribution of inter-canopy gaps, soil texture and crusting information on rangelands and pasture lands across North America. The BLM implements AIM on more than 247.3 million acres of land across the western US, encompassing major dust source regions of the Chihuahuan, Sonoran, Mojave and Great Basin deserts, the Colorado Plateau, and potential high-latitude dust sources in Alaska. The AIM data are publicly available and can be used to support modeling of land surface and boundary-layer processes, including dust emission. While understanding US dust source regions and emission processes has been of national interest since the 1930s Dust Bowl, most attention has been directed to the croplands of the Great Plains and emission hot spots like Owens Lake, California. The magnitude, spatial extent and temporal dynamics of dust emissions from western dust source areas remain highly uncertain. Here, we use ensemble modeling with empirical and physically-based dust emission schemes applied to AIM monitoring data to assess regional-scale patterns of aeolian sediment mass fluxes and dust emissions. The analysis enables connections to be made between dust emission rates at source and other indicators of ecosystem function at the landscape scale. Emerging ecological datasets like AIM provide new opportunities to evaluate aeolian sediment transport responses to land surface conditions, potential interactions with disturbances (e.g., fire) and ecological change (e.g., invasive species), and the impacts of anthropogenic land use and land cover change.

Mineral Dust Instantaneous Radiative Forcing in the Arctic

NASA Astrophysics Data System (ADS)

Kylling, A.; Groot Zwaaftink, C. D.; Stohl, A.

2018-05-01

Mineral dust sources at high and low latitudes contribute to atmospheric dust loads and dust deposition in the Arctic. With dust load estimates from Groot Zwaaftink et al. (https://doi.org/10.1002/2016JD025482), we quantify the mineral dust instantaneous radiative forcing (IRF) in the Arctic for the year 2012. The annual-mean top of the atmosphere IRF is 0.225 W/m2, with the largest contributions from dust transported from Asia south of 60°N and Africa. High-latitude (>60°N) dust sources contribute about 39% to top of the atmosphere IRF and have a larger impact (1 to 2 orders of magnitude) on IRF per emitted kilogram of dust than low-latitude sources. Mineral dust deposited on snow accounts for nearly all of the bottom of the atmosphere IRF of 0.135 W/m2. More than half of the bottom of the atmosphere IRF is caused by dust from high-latitude sources, indicating substantial regional climate impacts rarely accounted for in current climate models.

New directions: Mineral dust and ozone - Heterogeneous chemistry

NASA Astrophysics Data System (ADS)

Ramachandran, S.

2015-04-01

Aerosols, the tiny solid or liquid particles suspended in air and produced from natural sources and anthropogenic activities, continue to contribute the largest uncertainty to radiative forcing (IPCC, 2013). Aerosol particles give rise to radiative forcing directly through scattering and absorption of solar and infrared radiation in the atmosphere. Aerosols also give rise to indirect radiative forcing by modifying the cloud optical properties and lifetimes. Among the aerosol species mineral dust and black carbon cause a warming (positive forcing) while sulphate and sea salt cause a cooling (negative forcing) of the Earth-atmosphere system. In tropics and sub-tropics mineral dust is a major contributor to aerosol loading and optical thickness. The global source strength of dust aerosol varies significantly on spatial and temporal scales. The source regions of dust are mainly deserts, dry lake beds, and semi-arid regions, in addition to drier regions where vegetation has been reduced or soil surfaces that are disturbed by man made activities. Anthropogenic activities mainly related to agriculture such as harvesting, ploughing, overgrazing, and cement production and transport also produce mineral dust. An estimated 2500 terragram (Tg, 1012 g) of mineral dust is emitted into the atmosphere per year, and dominates the aerosol mass over continental regions in south Asia and China accounting for ∼35% of the total aerosol mass (IPCC, 2013). In India, dust is prevalent throughout the north and western India during the year and peaks during premonsoon season.

Harmattan, Saharan heat low, and West African monsoon circulation: modulations on the Saharan dust outflow towards the North Atlantic

NASA Astrophysics Data System (ADS)

Schepanski, Kerstin; Heinold, Bernd; Tegen, Ina

2017-09-01

The outflow of dust from the northern African continent towards the North Atlantic is stimulated by the atmospheric circulation over North Africa, which modulates the spatio-temporal distribution of dust source activation and consequently the entrainment of mineral dust into the boundary layer, as well as the transport of dust out of the source regions. The atmospheric circulation over the North African dust source regions, predominantly the Sahara and the Sahel, is characterized by three major circulation regimes: (1) the harmattan (trade winds), (2) the Saharan heat low (SHL), and (3) the West African monsoon circulation. The strength of the individual regimes controls the Saharan dust outflow by affecting the spatio-temporal distribution of dust emission, transport pathways, and deposition fluxes.This study aims at investigating the atmospheric circulation pattern over North Africa with regard to its role favouring dust emission and dust export towards the tropical North Atlantic. The focus of the study is on summer 2013 (June to August), during which the SALTRACE (Saharan Aerosol Long-range TRansport and Aerosol-Cloud interaction Experiment) field campaign also took place. It involves satellite observations by the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) flying on board the geostationary Meteosat Second Generation (MSG) satellite, which are analysed and used to infer a data set of active dust sources. The spatio-temporal distribution of dust source activation frequencies (DSAFs) allows for linking the diurnal cycle of dust source activations to dominant meteorological controls on dust emission. In summer, Saharan dust source activations clearly differ from dust source activations over the Sahel regarding the time of day when dust emission begins. The Sahara is dominated by morning dust source activations predominantly driven by the breakdown of the nocturnal low-level jet. In contrast, dust source activations in the Sahel are predominantly activated during the second half of the day, when downdrafts associated with deep moist convection are the major atmospheric driver. Complementary to the satellite-based analysis on dust source activations and implications from their diurnal cycle, simulations on atmosphere and dust life cycle were performed using the mesoscale atmosphere-dust model system COSMO-MUSCAT (COSMO: COnsortium for Small-scale MOdelling; MUSCAT: MUltiScale Chemistry Aerosol Transport Model). Fields from this simulation were analysed regarding the variability of the harmattan, the Saharan heat low, and the monsoon circulation as well as their impact on the variability of the Saharan dust outflow towards the North Atlantic. This study illustrates the complexity of the interaction among the three major circulation regimes and their modulation of the North African dust outflow. Enhanced westward dust fluxes frequently appear following a phase characterized by a deep SHL. Ultimately, findings from this study contribute to the quantification of the interannual variability of the atmospheric dust burden.

Dust loading of the normal atmosphere

NASA Astrophysics Data System (ADS)

Hall, F. F., Jr.

1983-01-01

Soil dust can contribute to atmospheric turbidity over most of the globe. The major sources of this dust are in the world's arid regions, where loadings of over 1000 micrograms/cu m can occur during strong winds. Saharan dust transported across the Atlantic can produce loadings up to 100 micrograms/cu m in the Western Hemisphere. Asian sources yield springtime loadings of 5-10 micrograms/cu m at Midway Island. Other important sources of dust are agricultural plowing and vehicular traffic on graded roads. The U.S. air quality standard of 75 micrograms/cu m is often exceeded in rural areas.

Infrared Photometry of 487 Sources in the Inner Regions of NGC 5128 (Centaurus A)

NASA Astrophysics Data System (ADS)

Alonso, M. Victoria; Minniti, Dante

1997-04-01

We study the sources present in the inner 3 kpc region of NGC 5128 (Cen A), most of which are star clusters of different ages. Photometry of archival Hubble Space Telescope WFPC images (F675W filter) is complemented with IR photometry (JHK' filters) obtained with the IRAC2B infrared array camera at the ESO/MPI 2.2 m telescope. From IR color maps we divide the field into two regions: a clear region outside the dust lane, and an obscured region well inside the dust lane of NGC 5128. In the unreddened region there is a great variety of sources such as globular clusters, star associations, and H II regions. These sources are not individual stars, which would be too faint to be resolved from ground-based telescopes. The vast majority of IR sources in the reddened region, where the dust lane dominates, are not seen at all in the deep HST images. The presence of large amounts of differential extinction makes it difficult to evaluate them. In total, there are 372 objects detected in the inner region of NGC 5128. From them, 125 objects are detected both in IR and HST frames. There are 247 IR sources without optical counterparts (47 in the clear region and 200 in the dust lane). Accounting for the small volume sampled, there must be a total of ~500 sources with K < 18 in the dust lane region. The distribution of these sources is rather uniform and not particularly centrally concentrated. This fact suggests that the majority of them are located in a disk, as would be expected if they are young associations or clusters. The degree of background and foreground contamination is evaluated using observations of a nearby field. We found 115 IR sources in this field. The nucleus itself is invisible in deep optical images, but it is clearly identified in the IR. In the region just south of the nucleus the extinction must be larger than AK = 3. In the clear region, where the effect of the dust lane is negligible, we have identified some objects as intermediate-age clusters containing carbon stars. From color-magnitude diagrams we do not find evidence of very young clusters in this region. Such clusters might be fainter than our detection limit in JHK'. We measure metallicities for 42 globular clusters, confirming the presence of a metallicity gradient with Δ[Fe/H]/ΔR = -0.06 dex kpc-1. Based on observations collected at La Silla Observatory and on archival data of the NASA/ESA Hubble Space Telescope, which is operated by AURA, Inc., under NASA contract NAS 5-26555.

Regional variability in dust-on-snow processes and impacts in the Upper Colorado River Basin

USGS Publications Warehouse

Skiles, S. McKenzie; Painter, Thomas H.; Belnap, Jayne; Holland, Lacey; Reynolds, Richard L.; Goldstein, Harland L.; Lin, J.

2015-01-01

Dust deposition onto mountain snow cover in the Upper Colorado River Basin frequently occurs in the spring when wind speeds and dust emission peaks on the nearby Colorado Plateau. Dust loading has increased since the intensive settlement in the western USA in the mid 1880s. The effects of dust-on-snow have been well studied at Senator Beck Basin Study Area (SBBSA) in the San Juan Mountains, CO, the first high-altitude area of contact for predominantly southwesterly winds transporting dust from the southern Colorado Plateau. To capture variability in dust transport from the broader Colorado Plateau and dust deposition across a larger area of the Colorado River water sources, an additional study plot was established in 2009 on Grand Mesa, 150 km to the north of SBBSA in west central, CO. Here, we compare the 4-year (2010–2013) dust source, deposition, and radiative forcing records at Grand Mesa Study Plot (GMSP) and Swamp Angel Study Plot (SASP), SBBSA's subalpine study plot. The study plots have similar site elevations/environments and differ mainly in the amount of dust deposited and ensuing impacts. At SASP, end of year dust concentrations ranged from 0.83 mg g−1 to 4.80 mg g−1, and daily mean spring dust radiative forcing ranged from 50–65 W m−2, advancing melt by 24–49 days. At GMSP, which received 1.0 mg g−1 less dust per season on average, spring radiative forcings of 32–50 W m−2 advanced melt by 15–30 days. Remote sensing imagery showed that observed dust events were frequently associated with dust emission from the southern Colorado Plateau. Dust from these sources generally passed south of GMSP, and back trajectory footprints modelled for observed dust events were commonly more westerly and northerly for GMSP relative to SASP. These factors suggest that although the southern Colorado Plateau contains important dust sources, dust contributions from other dust sources contribute to dust loading in this region, and likely account for the majority of dust loading at GMSP.

High-latitude dust in the Earth system

USGS Publications Warehouse

Bullard, Joanna E; Baddock, Matthew; Bradwell, Tom; Crusius, John; Darlington, Eleanor; Gaiero, Diego; Gasso, Santiago; Gisladottir, Gudrun; Hodgkins, Richard; McCulloch, Robert; NcKenna Neuman, Cheryl; Mockford, Tom; Stewart, Helena; Thorsteinsson, Throstur

2016-01-01

Natural dust is often associated with hot, subtropical deserts, but significant dust events have been reported from cold, high latitudes. This review synthesizes current understanding of high-latitude (≥50°N and ≥40°S) dust source geography and dynamics and provides a prospectus for future research on the topic. Although the fundamental processes controlling aeolian dust emissions in high latitudes are essentially the same as in temperate regions, there are additional processes specific to or enhanced in cold regions. These include low temperatures, humidity, strong winds, permafrost and niveo-aeolian processes all of which can affect the efficiency of dust emission and distribution of sediments. Dust deposition at high latitudes can provide nutrients to the marine system, specifically by contributing iron to high-nutrient, low-chlorophyll oceans; it also affects ice albedo and melt rates. There have been no attempts to quantify systematically the expanse, characteristics, or dynamics of high-latitude dust sources. To address this, we identify and compare the main sources and drivers of dust emissions in the Northern (Alaska, Canada, Greenland, and Iceland) and Southern (Antarctica, New Zealand, and Patagonia) Hemispheres. The scarcity of year-round observations and limitations of satellite remote sensing data at high latitudes are discussed. It is estimated that under contemporary conditions high-latitude sources cover >500,000 km2 and contribute at least 80–100 Tg yr−1 of dust to the Earth system (~5% of the global dust budget); both are projected to increase under future climate change scenarios.

High Latitude Dust in the Earth System

NASA Technical Reports Server (NTRS)

Bullard, Joanna E.; Baddock, Matthew; Bradwell, Tom; Crusius, John; Darlington, Eleanor; Gaiero, Diego; Gasso, Santiago; Gisladottir, Gudrun; Hodgkins, Richard; McCulloch, Robert;

Dust as a tipping element: The Bodélé Depression, Chad

PubMed Central

Washington, Richard; Bouet, Christel; Cautenet, Guy; Mackenzie, Elisabeth; Ashpole, Ian; Engelstaedter, Sebastian; Lizcano, Gil; Henderson, Gideon M.; Schepanski, Kerstin; Tegen, Ina

2009-01-01

Dust plays a vital role in climate and biophysical feedbacks in the Earth system. One source of dust, the Bodélé Depression in Chad, is estimated to produce about half the mineral aerosols emitted from the Sahara, which is the world's largest source. By using a variety of new remote sensing data, regional modeling, trajectory models, chemical analyses of dust, and future climate simulations, we investigate the current and past sensitivity of the Bodélé. We show that minor adjustments to small features of the atmospheric circulation, such as the Bodélé Low-Level Jet, could profoundly alter the behavior of this feature. Dust production during the mid-Holocene ceased completely from this key source region. Although subject to a great deal of uncertainty, some simulations of the 21st century indicate the potential for a substantial increase in dust production by the end of the century in comparison with current values. PMID:19620716

High concentrations of regional dust from deserts to plains across the central Rocky Mountains, USA

NASA Astrophysics Data System (ADS)

Reynolds, R. L.; Munson, S. M.; Fernandez, D. P.; Neff, J. C.

2015-12-01

Regional mineral dust in the American Southwest affects snow-melt rates, biogeochemical cycling, visibility, and public health. We measured total suspended particulates (TSP) across a 500-km-long sampling network of five remote sites in Utah and Colorado, USA, forming a gradient in distance from major dust emitting areas. The two westernmost sites on the Colorado Plateau desert had similar TSP concentrations (2008-2012, daily average=126 μg m-3; max. daily average over a two-week period=700 μg m-3 at Canyonlands National Park, Utah), while the easternmost High Plains site, close to cropped and grazed areas in northeastern Colorado, had an average concentration of 143 μg m-3 in 2011-2012 (max. daily average=656 μg m-3). Such concentrations rank comparably with those of TSP in several African and Asian cities in the paths of frequent dust storms. Dust loadings at the two intervening montane sites decreased from the western slope of the Rocky Mountains (Telluride, daily average=68 μg m-3) to an eastern site (Niwot Ridge, daily average=58 μg m-3). Back-trajectory analyses and satellite retrievals indicated that the three westernmost sites received most dust from large desert-source regions as far as 300 km to their southwest. These sources also sometimes sent dust to the two easternmost sites, which additionally captured dust from sources north and northwest of the central Rocky Mountains as well as locally at the Plains site. The PM10 fraction accounted for <15% of TSP, but most TSP is only slightly larger (typical median size, 15-20 μm) after about 100-800 km transport distances. Correlations between TSP and PM10 values indicate increases in both fractions during regional wind storms, especially related to Pacific frontal systems during late winter to late spring. These measurements and observations indicate that most dust deposition and associated air-quality problems in the interior American West are connected to regional dust sources and not to those in Asia.

Geochemical evidence for diversity of dust sources in the southwestern United States

USGS Publications Warehouse

Reheis, M.C.; Budahn, J.R.; Lamothe, P.J.

2002-01-01

Several potential dust sources, including generic sources of sparsely vegetated alluvium, playa deposits, and anthropogenic emissions, as well as the area around Owens Lake, California, affect the composition of modern dust in the southwestern United States. A comparison of geochemical analyses of modern and old (a few thousand years) dust with samples of potential local sources suggests that dusts reflect four primary sources: (1) alluvial sediments (represented by Hf, K, Rb, Zr, and rare-earth elements, (2) playas, most of which produce calcareous dust (Sr, associated with Ca), (3) the area of Owens (dry) Lake, a human-induced playa (As, Ba, Li, Pb, Sb, and Sr), and (4) anthropogenic and/or volcanic emissions (As, Cr, Ni, and Sb). A comparison of dust and source samples with previous analyses shows that Owens (dry) Lake and mining wastes from the adjacent Cerro Gordo mining district are the primary sources of As, Ba, Li, and Pb in dusts from Owens Valley. Decreases in dust contents of As, Ba, and Sb with distance from Owens Valley suggest that dust from southern Owens Valley is being transported at least 400 km to the east. Samples of old dust that accumulated before European settlement are distinctly lower in As, Ba, and Sb abundances relative to modern dust, likely due to modern transport of dust from Owens Valley. Thus, southern Owens Valley appears to be an important, geochemically distinct, point source for regional dust in the southwestern United States. Copyright ?? 2002 Elsevier Science Ltd.

Physical and Chemical Characteristics of Desert Dust Deposited on Mt. Elbrus, Caucasus as Documented in Snow Pit and Shallow Core Records

NASA Astrophysics Data System (ADS)

Kutuzov, S.; Shahgedanova, M.; Mikhalenko, V.; Ginot, P.; Lavrentiev, I.; Popov, G.

2013-12-01

We present a study of dust deposition events and its physical and chemical characteristics in Caucasus Mountains as documented by snow and firn pack at Mt Elbrus. Dust samples were collected from the shallow ice cores and snow pits in 2009-2013 at the western Elbrus plateau (5150 m a.s.l.). Particle size distribution and chemical analysis (major ions, trace elements) were completed for each sample using Coulter Counter Multisizer III, scanning electron microscopy (SEM), IC and ICPMS analysis. It was shown that desert dust deposition occurred in Caucasus 4-8 times a year and originates from the Northern Sahara and the deserts of the Middle East. Analysis of volumetric particle size distributions showed that the modal values ranged between 2 μm and 4 μm although most samples were characterised by modal values of 2.0-2.8 μm with an average of 2.6 μm. These values are lower than those obtained from the ice cores in central and southern Asia following the deposition of long-travelled dust and are closer to those reported for the European Alps and the polar ice cores. All samples containing dust have a single mode which is usually interpreted as a single source region. They do not reveal any significant differences between the Saharan and the Middle Eastern sources. The annual average dust mass concentrations were 10-15 mg kg-1 which is higher than the average concentrations reported for other mountain regions and this was strongly affected by dust deposition events. The deposition of dust resulted in elevated concentrations of most ions, especially Ca2+, Mg2+, K+, and sulphates. Dust originated from multiple sources in the Middle East including Mesopotamia or passing over the Middle East was characterised by the elevated concentrations of nitrates and ammonia which is related to a high atmospheric loads of ammonium emitted by agricultural sources and high concentrations of ammonium in dust originating from this region. By contrast, samples of the Saharan dust showed low concentrations consistent with the low ammonium loads in the source region. . The research leading to these results has received funding from the European Union Seventh Framework Programme FP7-PEOPLE-2010-IIF under grant agreement PIIF-GA-2010-275071 Russian Foundation for Basic Research (grants 11-05-00304 and 13-05-10069).

Characterisation of mineral dust emission in the Middle EAST using the Spinning Enhanced Visible and Infrared Imager (SEVIRI)

NASA Astrophysics Data System (ADS)

Hennen, M.; Shahgedanova, M.; White, K.

2015-12-01

Using the Spinning Enhanced Visual and InfraRed Imager (SEVIRI) on-board Meteosat's second generation satellite (MSG), mineral dust emissions from the Middle East were observed at a high temporal and spatial resolution between the years 2006 and 2013. This research provides a subjective derivation of mineral dust source locations in the Middle East using the thermal infrared Dust RGB product. Focusing on the brightness temperature difference around 10.8 µm channel and their spectral contrast with clear sky conditions, the Dust RGB product has been recognised as a major asset in detecting dust. While the product has already been used to map dust emissions in Sahara and south Africa, this research is the first to map dust emissions in the Middle East using SEVIRI, one of the dustiest regions in the world second only to the Sahara Desert. For every dust storm activation within the Middle East, the point of first emission is derived from visual inspection of each 15 minute image, these points were then recorded in a dust source climatology (DSC) database, along with time and direction of dust movement. To take account of potential errors inherent in this subjective detection method, a degree of confidence is associated with each data point with relevance to time of day (which has a strong effect on ability to detect dust in these products) and weather conditions, in particular presence of clouds. These results are compared with an automated retrieval using Aerosol Optical Depth (AOD) measurements form the Moderate Resolution Image Spectrometer (MODIS); which, due to its sun-synchronous orbit allows a measurement of dust in the atmosphere once a day. Differences in the spatial distribution of SEVIRI dust sources and MODIS inferred dust source regions can be explained by inherent transport bias in the latter's low sampling rate and prevailing wind conditions. This database will provide an important tool in further understanding dust emission processes in the region, laying the foundations for future studies relating to climatic conditions, especially droughts, and changes in land cover.

Global Distributions of Mineral Dust Properties from SeaWiFS and MODIS: From Sources to Sinks

NASA Technical Reports Server (NTRS)

Hsu, N. Christina; Bettenhausen, C.; Sayer, A.

2011-01-01

The impact of natural and anthropogenic sources of mineral dust has gained increasing attention from scientific communities in recent years. Indeed, these airborne dust particles, once lifted over the source regions, can be transported out of the boundary layer into the free troposphere and can travel thousands of kilometers across the oceans resulting in important biogeochemical impacts on the ecosystem. Due to the relatively short lifetime (a few hours to about a week), the distributions of these mineral dust particles vary extensively in both space and time. Consequently, satellite observations are needed over both source and sink regions for continuous temporal and spatial sampling of aerosol properties. With the launch of SeaWiFS in 1997, Terra/MODIS in 1999, and Aqua/MODIS in 2002, high quality comprehensive aerosol climatology is becoming feasible for the first time. As a result of these unprecedented satellite data records, studies of the radiative and biogeochemical effects due to dust aerosols are now possible. In this study, we will show the comparisons of satellite retrieved aerosol optical thickness using Deep Blue algorithm with data from AERONET sunphotometers over desert and semi-desert regions as well as vegetated areas. Our results indicate reasonable agreements between these two. These new satellite products will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from Sea WiFS and MODIS-like instruments. The multiyear satellite measurements since 1997 from Sea WiFS will be compared with those retrieved from MODIS and MISR, and will be utilized to investigate the interannual variability of source, pathway, and dust loading associated with the dust outbreaks over the entire globe. Finally, the trends observed over the last decade based upon the SeaWiFS time series in the amounts of tropospheric aerosols due to natural and anthropogenic sources (such as changes in the frequency of dust storms) will be discussed.

An Isotopic Map of Dust Source Areas in the McMurdo Sound Sector of Antarctica

NASA Astrophysics Data System (ADS)

Blakowski, M. A.; Aciego, S.; Delmonte, B.; Baroni, C.; Salvatore, M. C.

2014-12-01

The McMurdo Sound sector of Antarctica features a unique, polar desert ecosystem characterized by low temperatures, hyper-aridity, and high-speed winds. These climatic conditions result in limited water sources, sparse vegetation, underdeveloped soils, and abundant unconsolidated sediment easily influenced by wind-driven transport. Radiogenic isotopes (87Sr/86Sr, 143Nd/144Nd) provide constant signatures of dust from source- to sink-areas. Accordingly, aeolian dust derived from arid regions has been recognized in many studies as an important tracer of atmospheric circulation, as well as a tool for deciphering past climatic conditions in dust source regions. However, while major global dust sources (e.g. from South America, Africa, and Asia) are well studied and easily identifiable via distinct isotopic signatures when encountered in different depositional environments (e.g. Antarctic ice cores), local material from sources in and around the ice-free Dry Valleys and surrounding areas have remained in need of further documentation. We analyzed 40 samples of silt, sand, glacial drift, and weathered regolith material in both fine (<5μm) and coarse fractions collected from Victoria Land and the McMurdo Sound sector, including Cape Royds, Cape Bird, and the McMurdo Ice Shelf. Here we present an ArcGIS-generated, high-precision geochemical map of Antarctic PSAs synthesized from our data and combined with geomorphological and stratigraphic information on the studied sites. We believe that our expanded isotopic catalogue and map can be used to enhance and/or prompt regional studies in a variety of disciplines, such as by providing greater constraints on models of regional dust variability and transport pathways and of the melting history of the Antarctic ice sheet, and by determining the provenance of dust archived in ice cores, lake sediment, soil records, and impurities in Antarctic sea-ice.

Trans boundary transport of pollutants by atmospheric mineral dust.

PubMed

Erel, Yigal; Dayan, Uri; Rabi, Reut; Rudich, Yinon; Stein, Mordechai

2006-05-01

The transport of anthropogenic pollution by desert dust in the Eastern Mediterranean region was studied by analyzing major and trace element composition, organic species, and Pb isotope ratios in suspended dust samples collected in Jerusalem, Israel. Dust storms in this region are associated with four distinct synoptic conditions (Red Sea Trough (RS), Eastern High (EH), Sharav Cyclone (SC), and Cold Depression (Cyprus low, CD)) that carry dust mostly from North African (SC, CD, EH) and Arabian and Syrian (RS, EH) deserts. Substantial contamination of dust particles by Pb, Cu, Zn, and Ni is observed, while other elements (Na, Ca, Mg, Mn, Sr, Rb, REE, U, and Th) display natural concentrations. Sequential extraction of the abovementioned elements from the dust samples shows that the carbonate and sorbed fractions contain most of the pollution, yet the Al-silicate fraction is also contaminated, implying that soils and sediments in the source terrains of the dust are already polluted. We identified the pollutant sources by using Pb isotopes. It appears that before the beginning of the dust storm, the pollutants in the collected samples are dominated by local sources but with the arrival of dust from North Africa, the proportion of foreign pollutants increases. Organic pollutants exhibit behavior similar and complementary to that of the inorganic tracers, attesting to the importance of anthropogenic-pollutant addition en route of the dust from its remote sources. Pollution of suspended dust is observed under all synoptic conditions, yet it appears that easterly winds carry higher proportions of local pollution and westerly winds carry pollution emitted in the Cairo basin. Therefore, pollution transport by mineral dust should be accounted for in environmental models and in assessing the health-related effects of mineral dust.

A 37,000-year environmental magnetic record of aeolian dust deposition from Burial Lake, Arctic Alaska

NASA Astrophysics Data System (ADS)

Dorfman, J. M.; Stoner, J. S.; Finkenbinder, M. S.; Abbott, M. B.; Xuan, C.; St-Onge, G.

2015-11-01

Environmental magnetism and radiocarbon dating of Burial Lake sediments constrain the timing and magnitude of regional aeolian deposition for the Noatak region of western Arctic Alaska for the last ∼37,000 years. Burial Lake (68.43°N, 159.17°W, 21.5 m water depth) is optimally located to monitor regional dust deposition because it is perched above local drainage and isolated from glacial processes. Cores collected in the summer of 2010 were studied through the application of magnetizations and progressive alternating field (AF) demagnetization of u-channel samples, with additional data provided by computed tomography (CT) derived density, hysteresis measurements, isothermal remanent magnetization (IRM) acquisition experiments, organic carbon content, biogenic silica, physical grain size, radiocarbon dating of wood, seeds, and plant macrofossils, point source magnetic susceptibility, and X-ray fluorescence (XRF). With similar magnetic properties to regional Alaskan loess deposits, low coercivity, highly magnetic material deposited during the late-Pleistocene contrasts with a high coercivity, weakly magnetic component found throughout the record, consistent with locally-derived detritus. The relative proportion of low coercivity to high coercivity magnetic material, defined by the S-Ratios, is used to reconstruct the regional input of dust to the basin over time. A four-fold decrease in the low coercivity component through the deglacial transition is interpreted to reflect diminished dust input to the region. Comparisons with potential sources of dust show that the timing of deposition in Burial Lake is largely consistent with general aridity, lack of vegetative cover, and increased windiness, rather than glacial advances or retreats. The influence from subaerial exposure of continental shelves cannot be ruled out as a significant far-field source of dust to interior Alaska during the Last Glacial Maximum (LGM), but is unlikely to have been the sole source, or to have contributed to increased dust in both the early and late Holocene.

Observations and Measurements of Dust Transport from the Patagonia Desert into the South Atlantic Ocean in 2004 and 2005

NASA Astrophysics Data System (ADS)

Gasso, S.; Gaiero, D. M.; Villoslada, B.; Liske, E.

2005-12-01

The largest continental landmass south of the 40-degree parallel and potentially one of the largest sources of dust into the Southern Ocean (SO) is the Patagonia desert. Most of the estimates of dust outflow and deposition from this region into the South Atlantic Ocean are based on model simulations. However, there are very few measurements available that can corroborate these estimates. Satellite assessments of dust activity offer conflicting views. For example, monthly time series of satellite-derived (e.g. AVHRR and MODIS) aerosol optical depth (AOD) indicate that dust activity is minimal. However, a study with the TOMS Aerosol Index (Prospero et al., 2002) showed that the frequency of dust events is in the range of 7-14 days/month during the years 1978 through 1993. In addition, surface visibility observations along the Patagonian coast confirm that ocean-going dust events do occur during the summer and spring months. These discrepancies indicate fundamental uncertainties regarding the frequency and extent of dust activity in Patagonia. Given that the SO is the largest high-chlorophyll, low-nutrient area in the world and that the flux of nutrient-rich dust has the potential to modify biological activity with possible climatic consequences, it is of interest to have a better understanding of how often and intense are dust events in the Patagonia region. We surveyed the reports of dust activity from surface weather stations in the Patagonia region during the period June, 2004 to April, 2005. These observations were compared with simultaneous MODIS true color pictures and the corresponding aerosol retrievals. In addition, measurements of vertical and horizontal dust flux were collected by dust samplers at four sites along the coast. The horizontal flux measurements were compared with the same estimates derived from MODIS. According to the true color pictures and confirmed by the surface visibility observations, we recorded at least 16 ocean-going dust events. The scale of the events varied from small (single dust plumes along the coast) to large (dust front extending ~600 km). Most of the large events occurred during the late summer. Due to the presence of sun glint, cloud obstruction, or coastal sediments, the MODIS automatic aerosol algorithm did not derive AODs in many instances and, as result, many events were not recorded in the MODIS monthly database. Dust sources are numerous and dust plumes outflow at any place along the coastline (> 1000 km) including some very active sources as far south as in the Tierra del Fuego Island (54S). The main sources identified are coastal saltbeds, inland deflation hollows and receding shores of large lakes. Although some of major emitting points have been included as sources in dust models, there are some notable exceptions, for example most of the coastal sources. We note, in addition, that the scale and diversity of the different sources pose significant challenges with respect to parameterization in global models of dust dispersion.

Spatial and Temporal Dust Source Variability in Northern China Identified Using Advanced Remote Sensing Analysis

NASA Technical Reports Server (NTRS)

Taramelli, A.; Pasqui, M.; Barbour, J.; Kirschbaum, D.; Bottai, L.; Busillo, C.; Calastrini, F.; Guarnieri, F.; Small, C.

2013-01-01

The aim of this research is to provide a detailed characterization of spatial patterns and temporal trends in the regional and local dust source areas within the desert of the Alashan Prefecture (Inner Mongolia, China). This problem was approached through multi-scale remote sensing analysis of vegetation changes. The primary requirements for this regional analysis are high spatial and spectral resolution data, accurate spectral calibration and good temporal resolution with a suitable temporal baseline. Landsat analysis and field validation along with the low spatial resolution classifications from MODIS and AVHRR are combined to provide a reliable characterization of the different potential dust-producing sources. The representation of intra-annual and inter-annual Normalized Difference Vegetation Index (NDVI) trend to assess land cover discrimination for mapping potential dust source using MODIS and AVHRR at larger scale is enhanced by Landsat Spectral Mixing Analysis (SMA). The combined methodology is to determine the extent to which Landsat can distinguish important soils types in order to better understand how soil reflectance behaves at seasonal and inter-annual timescales. As a final result mapping soil surface properties using SMA is representative of responses of different land and soil cover previously identified by NDVI trend. The results could be used in dust emission models even if they are not reflecting aggregate formation, soil stability or particle coatings showing to be critical for accurately represent dust source over different regional and local emitting areas.

East Asian origin of central Greenland last glacial dust: just one possible scenario?

NASA Astrophysics Data System (ADS)

Újvári, Gábor; Stevens, Thomas; Svensson, Anders; Klötzli, Urs Stephan; Manning, Christina; Németh, Tibor; Kovács, János

2016-04-01

Dust in Greenland ice cores is used to reconstruct the activity of dust emitting regions and atmospheric circulation for the last glacial period. However, the source dust material to Greenland over this period is the subject of considerable uncertainty. Here we use new clay mineral and Sr-Nd isotopic data from eleven loess samples collected around the Northern Hemisphere and compare the 87Sr/86Sr and 143Nd/144Nd isotopic signatures of fine (<10 μm) separates to existing Greenland ice core dust data (GISP2, GRIP; [1]; [2]). Smectite contents and kaolinite/chlorite (K/C) ratios allow exclusion of continental US dust emitting regions as potential sources, because of the very high (>3.6) K/C ratios and extremely high (>~70%) smectite contents. At the same time, Sr-Nd isotopic compositions demonstrate that ice core dust isotopic compositions can be explained by East Asian (Chinese loess) and/or Central/East Central European dust contributions. Central/East Central European loess Sr-Nd isotopic compositions overlap most with ice core dust, while the Sr isotopic signature of Chinese loess is slightly more radiogenic. Nevertheless, an admixture of 90‒10 % from Chinese loess and circum-Pacific volcanic material would also account for the Sr‒Nd isotopic ratios of central Greenland LGM dust. At the same time, sourcing of ice core dust from Alaska, continental US and NE Siberia seems less likely based on Sr and Nd isotopic signatures. The data demonstrate that currently no unique source discrimination for Greenland dust is possible using both published and our new data [3]. Thus, there is a need to identify more diagnostic tracers. Based on initial Hf isotope analyses of fine separates of three loess samples (continental US, Central Europe, China), an apparent dependence of Hf isotopic signatures on the relative proportions of radiogenic clay minerals (primarily illite) was found, as these fine dust fractions are apparently zircon-free. The observed difference between major potential source regions in 176Hf/177Hf that reach several ɛHf units and the first order clay mineralogy dependence of Hf isotopic signatures means there is strong potential for distinguishing between the two hypothesized Greenland dust sources using Hf isotopes [3]. [1] Biscaye P.E., Grousset F.E., Revel M., Van der Gaast S., Zielinski G.A., Vaars A., Kukla G. (1997). Asian provenance of glacial dust (stage 2) in the Greenland Ice Sheet Project 2 Ice Core, Summit, Greenland. Journal of Geophysical Research 102, 26765-26781. [2] Svensson A., Biscaye P.E., Grousset F.E. (2000) Characterization of late glacial continental dust in the Greenland Ice Core Project ice core. Journal of Geophysical Research 105, 4637-4656. [3] Újvári G., Stevens T., Svensson A., Klötzli U.S., Manning, C., Németh T., Kovács J., Sweeney M.R., Gocke M., Wiesenberg G.L.B., Markovic S.B., Zech M. (in press). Two possible source regions for Central Greenland last glacial dust. Geophysical Research Letters, doi: 10.1002/2015GL066153.

Estimation of global anthropogenic dust aerosol using CALIOP satellite

NASA Astrophysics Data System (ADS)

Chen, B.; Huang, J.; Liu, J.

2014-12-01

Anthropogenic dust aerosols are those produced by human activity, which mainly come from cropland, pasture, and urban in this paper. Because understanding of the emissions of anthropogenic dust is still very limited, a new technique for separating anthropogenic dust from natural dustusing CALIPSO dust and planetary boundary layer height retrievalsalong with a land use dataset is introduced. Using this technique, the global distribution of dust is analyzed and the relative contribution of anthropogenic and natural dust sources to regional and global emissions are estimated. Local anthropogenic dust aerosol due to human activity, such as agriculture, industrial activity, transportation, and overgrazing, accounts for about 22.3% of the global continentaldust load. Of these anthropogenic dust aerosols, more than 52.5% come from semi-arid and semi-wet regions. On the whole, anthropogenic dust emissions from East China and India are higher than other regions.

Asian anthropogenic dust and its climate effect (Invited)

NASA Astrophysics Data System (ADS)

Huang, J.; Liu, J.; Chen, B.

2013-12-01

Anthropogenic dust originates mainly from areas of localized human disturbance, such as traffic-on-roads, agricultural fields, grazing, military installations, construction sites, and off-road vehicle areas. To understand historical and possible future changes in dust emissions, the percentage of atmospheric dust load originating from anthropogenic source and its distribution must be quantified. CALIPSO lidar, which shoots a laser into the atmosphere, provides new insight into the detection of anthropogenic dust emission. Here, we present the distribution of Asian anthropogenic dust emissions and its relation to human activity by using CALIPSO lidar measurements. We found that the local anthropogenic dust aerosols account for significant portion of the total dust burden in the atmosphere. The anthropogenic dust emissions mainly occur over the heavy human activity and poor ecosystem region, such as semi-arid region. The impact of Asian anthropogenic dust on regional climate will also be discussed in this talk.

Glacial/interglacial changes of Southern Hemisphere wind circulation from the geochemistry of South American dust

NASA Astrophysics Data System (ADS)

Gili, Stefania; Gaiero, Diego M.; Goldstein, Steven L.; Chemale, Farid; Jweda, Jason; Kaplan, Michael R.; Becchio, Raúl A.; Koester, Edinei

2017-07-01

The latitudinal displacement of the southern westerlies and associated climate systems is a key parameter for understanding the variations of Southern Hemisphere atmospheric circulation during the Late Quaternary Period. To increase understanding of past atmospheric circulation and of the paleo-environmental conditions associated with continental dust sources, we dig deeper into dust provenance in paleo-archives of the Southern Hemisphere. We present here a Sr-Nd isotopic and rare earth element study of surface sediments collected along a ∼4000 km latitudinal band from arid and semi-arid terrains in southern South America. Findings from terrains that served as paleo-dust suppliers are compared with modern dust collected from monitoring stations along the same latitudinal band, which affords a test on how actual present-day aeolian compositions compare to those of the past potential source areas. Moreover, the comparison between past and present-day datasets is useful for understanding present-day atmospheric circulation. Armed with a new comprehensive dataset, we revise previous interpretations of the provenance of dust trapped in the Antarctic ice and sediments deposited in the South Atlantic sector of the Southern Ocean. These comparisons support multiple source regions in southern South America that changed with climates. The findings reveal that, although Patagonia plays an important role in contributing dust to the higher latitudes, central Western Argentina and (to a lesser extent) the southern Puna region also emerge as potentially important dust sources during glacial times. The southern Altiplano appears to be a major contributor during interglacial periods as well. We rely in part on an understanding of modern wind-dust activities to conclude that the possible presence of southern South America source regions - other than Patagonia - in East Antarctic ice is consistent with an overall equatorward displacement during glacial times of both the mid-latitude westerlies and the subtropical jet stream.

NHEXAS PHASE I REGION 5 STUDY--METALS IN DUST ANALYTICAL RESULTS

EPA Science Inventory

This data set includes analytical results for measurements of metals in 1,906 dust samples. Dust samples were collected to assess potential residential sources of dermal and inhalation exposures and to examine relationships between analyte levels in dust and in personal and bioma...

Urban dust in the Guanzhong basin of China, part II: A case study of urban dust pollution using the WRF-Dust model.

PubMed

Li, Nan; Long, Xin; Tie, Xuexi; Cao, Junji; Huang, Rujin; Zhang, Rong; Feng, Tian; Liu, Suixin; Li, Guohui

2016-01-15

We developed a regional dust dynamical model (WRF-Dust) to simulate surface dust concentrations in the Guanzhong (GZ) basin of China during two typical dust cases (19th Aug. and 26th Nov., 2013), and compared model results with the surface measurements at 17 urban and rural sites. The important improvement of the model is to employ multiple high-resolution (0.5-500 m) remote sensing data to construct dust sources. The new data include the geographic information of constructions, croplands, and barrens over the GZ basin in summer and winter of 2013. For the first time, detailed construction dust emissions have been introduced in a regional dust model in large cities of China. Our results show that by including the detailed dust sources, model performance at simulating dust pollutions in the GZ basin is significantly improved. For example, the simulated dust concentration average for the 17 sites increases from 28 μg m(-3) to 59 μg m(-3), closing to the measured concentration of 66 μg m(-3). In addition, the correlation coefficient (r) between the calculated and measured dust concentrations is also improved from 0.17 to 0.57, suggesting that our model better presents the spatial variation. Further analysis shows that urban construction activities are the crucial source in controlling urban dust pollutions. It should be considered by policy makers for mitigating particulate air pollution in many Chinese cities. Copyright © 2015 Elsevier B.V. All rights reserved.

Profiling of Saharan dust from the Caribbean to western Africa - Part 2: Shipborne lidar measurements versus forecasts

NASA Astrophysics Data System (ADS)

Ansmann, Albert; Rittmeister, Franziska; Engelmann, Ronny; Basart, Sara; Jorba, Oriol; Spyrou, Christos; Remy, Samuel; Skupin, Annett; Baars, Holger; Seifert, Patric; Senf, Fabian; Kanitz, Thomas

2017-12-01

A unique 4-week ship cruise from Guadeloupe to Cabo Verde in April-May 2013 see part 1, Rittmeister et al. (2017) is used for an in-depth comparison of dust profiles observed with a polarization/Raman lidar aboard the German research vessel Meteor over the remote tropical Atlantic and respective dust forecasts of a regional (SKIRON) and two global atmospheric (dust) transport models (NMMB/BSC-Dust, MACC/CAMS). New options of model-observation comparisons are presented. We analyze how well the modeled fine dust (submicrometer particles) and coarse dust contributions to light extinction and mass concentration match respective lidar observations, and to what extent models, adjusted to aerosol optical thickness observations, are able to reproduce the observed layering and mixing of dust and non-dust (mostly marine) aerosol components over the remote tropical Atlantic. Based on the coherent set of dust profiles at well-defined distances from Africa (without any disturbance by anthropogenic aerosol sources over the ocean), we investigate how accurately the models handle dust removal at distances of 1500 km to more than 5000 km west of the Saharan dust source regions. It was found that (a) dust predictions are of acceptable quality for the first several days after dust emission up to 2000 km west of the African continent, (b) the removal of dust from the atmosphere is too strong for large transport paths in the global models, and (c) the simulated fine-to-coarse dust ratio (in terms of mass concentration and light extinction) is too high in the models compared to the observations. This deviation occurs initially close to the dust sources and then increases with distance from Africa and thus points to an overestimation of fine dust emission in the models.

Identifying sources of aeolian mineral dust: Present and past

USGS Publications Warehouse

Muhs, Daniel R; Prospero, Joseph M; Baddock, Matthew C; Gill, Thomas E

2014-01-01

Aeolian mineral dust is an important component of the Earth’s environmental systems, playing roles in the planetary radiation balance, as a source of fertilizer for biota in both terrestrial and marine realms and as an archive for understanding atmospheric circulation and paleoclimate in the geologic past. Crucial to understanding all of these roles of dust is the identification of dust sources. Here we review the methods used to identify dust sources active at present and in the past. Contemporary dust sources, produced by both glaciogenic and non-glaciogenic processes, can be readily identified by the use of Earth-orbiting satellites. These data show that present dust sources are concentrated in a global dust belt that encompasses large topographic basins in low-latitude arid and semiarid regions. Geomorphic studies indicate that specific point sources for dust in this zone include dry or ephemeral lakes, intermittent stream courses, dune fields, and some bedrock surfaces. Back-trajectory analyses are also used to identify dust sources, through modeling of wind fields and the movement of air parcels over periods of several days. Identification of dust sources from the past requires novel approaches that are part of the geologic toolbox of provenance studies. Identification of most dust sources of the past requires the use of physical, mineralogical, geochemical, and isotopic analyses of dust deposits. Physical properties include systematic spatial changes in dust deposit thickness and particle size away from a source. Mineralogy and geochemistry can pinpoint dust sources by clay mineral ratios and Sc-Th-La abundances, respectively. The most commonly used isotopic methods utilize isotopes of Nd, Sr, and Pb and have been applied extensively in dust archives of deep-sea cores, ice cores, and loess. All these methods have shown that dust sources have changed over time, with far more abundant dust supplies existing during glacial periods. Greater dust supplies in glacial periods are likely due to greater production of glaciogenic dust particles from expanded ice sheets and mountain glaciers, but could also include dust inputs from exposed continental and insular shelves now submerged. Future dust sources are difficult to assess, but will likely differ from those of the present because of global warming. Global warming could bring about shifts in dust sources by changes in degree or type of vegetation cover, changes in wind strength, and increases or decreases in the size of water bodies. A major uncertainty in assessing dust sources of the future is related to changes inhuman land use, which could affect land surface cover, particularly due to increased agricultural endeavors and water usage.

Climatology of dust distribution over West Asia from homogenized remote sensing data

NASA Astrophysics Data System (ADS)

Nabavi, Seyed Omid; Haimberger, Leopold; Samimi, Cyrus

2016-06-01

In the past decade, West Asia has witnessed more frequent and intensified dust storms affecting Iran and Persian Gulf countries. Employing a varying threshold that takes into account systematic differences between TOMS and OMI data, TOMS-OMI Aerosol Index data are used to identify long-term changes in the horizontal distribution of dust storms in West Asia from 1980 to present. The northwest of Iraq and east of Syria are identified as emerging dusty areas, whereas east of Saudi Arabia and southeast of Iraq are identified as permanent dusty areas, including both dust sources and affected areas. Whereas the frequency of dust events increased slightly in the permanent dusty areas, it increased markedly in the emerging dusty areas. As expected, the frequency of dust events is highest in June and July. The dust source areas are identified as the Iraq-Saudi Arabia boundary region and (recently) the northwest of Iraq, using MODIS deep blue aerosol optical depth data. Subsequently, a lagged correlation was implemented between identified dust sources and whole West Asia to determine the main paths and receptors of intense dust storms. Accordingly, southwest of Iran and Persian Gulf countries were determined as main receptors of summertime dust storms in West Asia. During spring, dust storms mostly hit the northern half of the region and reach to the Caspian Sea. Analyzing atmospheric patterns, Shamal and Frontal patterns were found as dominant atmospheric circulations simultaneous with summertime and springtime dust storms, respectively.

Probing the Interstellar Dust towards the Galactic Centre using X-ray Dust Scattering Halos

NASA Astrophysics Data System (ADS)

Jin, C.; Ponti, G.; Haberl, F.; Smith, R.

2017-10-01

Dust scattering creates an X-ray halo that contains abundant information about the interstellar dust along the source's line-of-sight (LOS), and is most prominent when the LOS nH is high. In this talk, I will present results from our latest study of a bright dust scattering halo around an eclipsing X-ray binary at 1.45 arcmin away from Sgr A*, namely AX J1745.6-2901. This study is based on a large set of XMM-Newton and Chandra observations, and is so-far the best dust scattering halo study of a X-ray transient in the Galactic centre (GC). I will show that the foreground dust of AX J1745.6-2901 can be decomposed into two major thick dust layers. One layer contains (66-81)% of the total LOS dust and is several kpc away from the source, and so is most likely to reside in the Galactic disc. The other layer is local to the source. I will also show that the dust scattering halo can cause the source spectrum to severely depend on the source extraction region. Such spectral bias can be corrected by our new Xspec model, which is likely to be applicable to Sgr A* and other GC sources as well.

Long-range transport and mixing of aerosol sources during the 2013 North American biomass burning episode: analysis of multiple lidar observations in the western Mediterranean basin

NASA Astrophysics Data System (ADS)

Ancellet, Gerard; Pelon, Jacques; Totems, Julien; Chazette, Patrick; Bazureau, Ariane; Sicard, Michaël; Di Iorio, Tatiana; Dulac, Francois; Mallet, Marc

2016-04-01

Long-range transport of biomass burning (BB) aerosols between North America and the Mediterranean region took place in June 2013. A large number of ground-based and airborne lidar measurements were deployed in the western Mediterranean during the Chemistry-AeRosol Mediterranean EXperiment (ChArMEx) intensive observation period. A detailed analysis of the potential North American aerosol sources is conducted including the assessment of their transport to Europe using forward simulations of the FLEXPART Lagrangian particle dispersion model initialized using satellite observations by MODIS and CALIOP. The three-dimensional structure of the aerosol distribution in the ChArMEx domain observed by the ground-based lidars (Minorca, Barcelona and Lampedusa), a Falcon-20 aircraft flight and three CALIOP tracks, agrees very well with the model simulation of the three major sources considered in this work: Canadian and Colorado fires, a dust storm from western US and the contribution of Saharan dust streamers advected from the North Atlantic trade wind region into the westerlies region. Four aerosol types were identified using the optical properties of the observed aerosol layers (aerosol depolarization ratio, lidar ratio) and the transport model analysis of the contribution of each aerosol source: (i) pure BB layer, (ii) weakly dusty BB, (iii) significant mixture of BB and dust transported from the trade wind region, and (iv) the outflow of Saharan dust by the subtropical jet and not mixed with BB aerosol. The contribution of the Canadian fires is the major aerosol source during this episode while mixing of dust and BB is only significant at an altitude above 5 km. The mixing corresponds to a 20-30 % dust contribution in the total aerosol backscatter. The comparison with the MODIS aerosol optical depth horizontal distribution during this episode over the western Mediterranean Sea shows that the Canadian fire contributions were as large as the direct northward dust outflow from Sahara.

Long range transport and mixing of aerosol sources during the 2013 North American biomass burning episode: analysis of multiple lidar observations in the Western Mediterranean basin

NASA Astrophysics Data System (ADS)

Ancellet, G.; Pelon, J.; Totems, J.; Chazette, P.; Bazureau, A.; Sicard, M.; Di Iorio, T.; Dulac, F.; Mallet, M.

2015-11-01

Long range transport of biomass burning (BB) aerosols between North America and the Mediterranean region took place in June 2013. A large number of ground based and airborne lidar measurements were deployed in the Western Mediterranean during the Chemistry-AeRosol Mediterranean EXperiment (ChArMEx) intensive observation period. A detailed analysis of the potential North American aerosol sources is conducted including the assessment of their transport to Europe using forward simulations of the FLEXPART Lagrangian particle dispersion model initialized using satellite observations by MODIS and CALIOP. The three dimensional structure of the aerosol distribution in the ChArMEx domain observed by the ground-based lidars (Menorca, Barcelona and Lampedusa), a Falcon-20 aircraft flight and three CALIOP tracks, agree very well with the model simulation of the three major sources considered in this work: Canadian and Colorado fires, a dust storm from Western US and the contribution of Saharan dust streamers advected from the North Atlantic trade wind region into the Westerlies region. Four aerosol types were identified using the optical properties of the observed aerosol layers (aerosol depolarization ratio, lidar ratio) and the transport model analysis of the contribution of each aerosol source: (I) pure BB layer, (II) weakly dusty BB, (III) significant mixture of BB and dust transported from the trade wind region (IV) the outflow of Saharan dust by the subtropical jet and not mixed with BB aerosol. The contribution of the Canadian fires is the major aerosol source during this episode while mixing of dust and BB is only significant at altitude above 5 km. The mixing corresponds to a 20-30 % dust contribution in the total aerosol backscatter. The comparison with the MODIS AOD horizontal distribution during this episode over the Western Mediterranean sea shows that the Canadian fires contribution were as large as the direct northward dust outflow from Sahara.

Sensitivity of surface characteristics on the simulation of wind-blown-dust source in North America

NASA Astrophysics Data System (ADS)

Park, S. H.; Gong, S. L.; Gong, W.; Makar, P. A.; Moran, M. D.; Stroud, C. A.; Zhang, J.

Recently, a wind-blown-dust-emission module has been built based on a state-of-the-art wind erosion theory and evaluated in a regional air-quality model to simulate a North American dust storm episode in April 2001 (see Park, S.H., Gong, S.L., Zhao, T.L., Vet, R.J., Bouchet, V.S., Gong, W., Makar, P.A., Moran, M.D., Stroud, C., Zhang, J. 2007. Simulation of entrainment and transport of dust particles within North America in April 2001 ("Red Dust episode"). J. Geophys. Res. 112, D20209, doi:10.1029/2007JD008443). A satisfactorily detailed assessment of that module, however, was not possible because of a lack of information on some module inputs, especially soil moisture content. In this paper, the wind-blown-dust emission was evaluated for two additional dust storms using improved soil moisture inputs. The surface characteristics of the wind-blown-dust source areas in southwestern North America were also investigated, focusing on their implications for wind-blown-dust emissions. The improved soil moisture inputs enabled the sensitivity of other important surface characteristics, the soil grain size distribution and the land-cover, to dust emission to be investigated with more confidence. Simulations of the two 2003 dust storm episodes suggested that wind-blown-dust emissions from the desert areas in southwestern North America are dominated by emissions from dry playas covered with accumulated alluvial deposits whose particle size is much smaller than usual desert sands. As well, the source areas in the northwestern Texas region were indicated to be not desert but rather agricultural lands that were "activated" as a wind-blown-dust sources after harvest. This finding calls for revisions to the current wind-blown-dust-emission module, in which "desert" is designated to be the only land-cover category that can emit wind-blown dust.

Characterization of aerosolized bacteria and fungi from desert dust events in Mali, West Africa

USGS Publications Warehouse

Kellogg, C.A.; Griffin, Dale W.; Garrison, V.H.; Peak, K.K.; Royall, N.; Smith, R.R.; Shinn, E.A.

2004-01-01

Millions of metric tons of African desert dust blow across the Atlantic Ocean each year, blanketing the Caribbean and southeastern United States. Previous work in the Caribbean has shown that atmospheric samples collected during dust events contain living microbes, including plant and opportunistic human pathogens. To better understand the potential downwind public health and ecosystem effects of the dust microbes, it is important to characterize the source population. We describe 19 genera of bacteria and 3 genera of fungi isolated from air samples collected in Mali, a known source region for dust storms, and over which large dust storms travel.

Characterizing Mineral Dust from the Arabian Coast of the Red Sea

NASA Astrophysics Data System (ADS)

Puthan Purakkal, J.; Stenchikov, G. L.; Engelbrecht, J. P.

2014-12-01

The Arabian Peninsula is one of the Earth's major sources of atmospheric dust. Along with profound negative effects on human activity and natural processes in this region, dust is an important nutrient source for the oligothrophic northern Red Sea. From preliminary observations it is estimated that some 18-20 major dust storms per year deposit about 6 Mt of mineral dust into the Red Sea. To better understand the optical properties, health, and ecological impacts of dust, we study the mineralogical, chemical and morphological properties of surface soil samples collected at prevbiously identified potential dust sources along the Arabian coast of the Red Sea. Many of these dust sources lie within a narrow coastal region and because of their proximity to the Red Sea, are important contributors to the dust/nutrient balance, during both dusty and fair weather conditions. Bulk samples were collected from the top 10 mm of soils from three sites along the Arabian coast of the Red Sea. The soil samples were sieved to separate the < 38μm particle fractions for chemical and mineralogical analysis. X-ray diffractometry (XRD) was applied to measure the mineral content of the dust. The chemical composition of individual particles was analyzed using scanning electron microscopy (SEM) with energy dispersive spectroscopy (EDS). From the XRD analysis of the sieved samples from An Masayat (23.3322 N, 38.9481 E), Buthna (23.2960 N, 38.9384 E) and Rabugh pipeline Road (23.292 N, 38.91 E), it was found that the dust was composed largely of hematite, goethite, calcite, dolomite, quartz, chlorite, muscovite, amphibole, epidote and plagioclase. Our results are being compared to, and show similarities to those of Engelbrecht et al. , collected at 15 Middle East sites. Both the mineralogical content and chemical composition of samples bear the signatures of the regional geology. Engelbrecht, J. P., McDonald, E. V., Gillies, J. A., Jayanty, R. K. M., Casuccio, G., and Gertler, A. W., 2009, Characterizing mineral dusts and other aerosols from the Middle East - Part 2: Grab samples and re-suspensions: Inhalation Toxicology, v. 21, p. 327-336.

Global Scale Attribution of Anthropogenic and Natural Dust Sources and their Emission Rates Based on MODIS Deep Blue Aerosol Products

NASA Technical Reports Server (NTRS)

Ginoux, Paul; Prospero, Joseph M.; Gill, Thomas E.; Hsu, N. Christina; Zhao, Ming

2012-01-01

Our understanding of the global dust cycle is limited by a dearth of information about dust sources, especially small-scale features which could account for a large fraction of global emissions. Here we present a global-scale high-resolution (0.1 deg) mapping of sources based on Moderate Resolution Imaging Spectroradiometer (MODIS) Deep Blue estimates of dust optical depth in conjunction with other data sets including land use. We ascribe dust sources to natural and anthropogenic (primarily agricultural) origins, calculate their respective contributions to emissions, and extensively compare these products against literature. Natural dust sources globally account for 75% of emissions; anthropogenic sources account for 25%. North Africa accounts for 55% of global dust emissions with only 8% being anthropogenic, mostly from the Sahel. Elsewhere, anthropogenic dust emissions can be much higher (75% in Australia). Hydrologic dust sources (e.g., ephemeral water bodies) account for 31% worldwide; 15% of them are natural while 85% are anthropogenic. Globally, 20% of emissions are from vegetated surfaces, primarily desert shrublands and agricultural lands. Since anthropogenic dust sources are associated with land use and ephemeral water bodies, both in turn linked to the hydrological cycle, their emissions are affected by climate variability. Such changes in dust emissions can impact climate, air quality, and human health. Improved dust emission estimates will require a better mapping of threshold wind velocities, vegetation dynamics, and surface conditions (soil moisture and land use) especially in the sensitive regions identified here, as well as improved ability to address small-scale convective processes producing dust via cold pool (haboob) events frequent in monsoon regimes.

The brightest high-latitude 12-micron IRAS sources

NASA Technical Reports Server (NTRS)

Hacking, P.; Beichman, C.; Chester, T.; Neugebauer, G.; Emerson, J.

1985-01-01

The Infrared Astronomical Satellite (IRAS) Point Source catalog was searched for sources brighter than 28 Jy (0 mag) at 12 microns with absolute galactic latitude greater than 30 deg excluding the Large Magellanic Cloud. The search resulted in 269 sources, two of which are the galaxies NGC 1068 and M82. The remaining 267 sources are identified with, or have infrared color indices consistent with late-type stars some of which show evidence of circumstellar dust shells. Seven sources are previously uncataloged stars. K and M stars without circumstellar dust shells, M stars with circumstellar dust shells, and carbon stars occupy well-defined regions of infrared color-color diagrams.

Global scale variability of the mineral dust long-wave refractive index: a new dataset of in situ measurements for climate modeling and remote sensing

NASA Astrophysics Data System (ADS)

Di Biagio, Claudia; Formenti, Paola; Balkanski, Yves; Caponi, Lorenzo; Cazaunau, Mathieu; Pangui, Edouard; Journet, Emilie; Nowak, Sophie; Caquineau, Sandrine; Andreae, Meinrat O.; Kandler, Konrad; Saeed, Thuraya; Piketh, Stuart; Seibert, David; Williams, Earle; Doussin, Jean-François

2017-02-01

Modeling the interaction of dust with long-wave (LW) radiation is still a challenge because of the scarcity of information on the complex refractive index of dust from different source regions. In particular, little is known about the variability of the refractive index as a function of the dust mineralogical composition, which depends on the specific emission source, and its size distribution, which is modified during transport. As a consequence, to date, climate models and remote sensing retrievals generally use a spatially invariant and time-constant value for the dust LW refractive index. In this paper, the variability of the mineral dust LW refractive index as a function of its mineralogical composition and size distribution is explored by in situ measurements in a large smog chamber. Mineral dust aerosols were generated from 19 natural soils from 8 regions: northern Africa, the Sahel, eastern Africa and the Middle East, eastern Asia, North and South America, southern Africa, and Australia. Soil samples were selected from a total of 137 available samples in order to represent the diversity of sources from arid and semi-arid areas worldwide and to account for the heterogeneity of the soil composition at the global scale. Aerosol samples generated from soils were re-suspended in the chamber, where their LW extinction spectra (3-15 µm), size distribution, and mineralogical composition were measured. The generated aerosol exhibits a realistic size distribution and mineralogy, including both the sub- and super-micron fractions, and represents in typical atmospheric proportions the main LW-active minerals, such as clays, quartz, and calcite. The complex refractive index of the aerosol is obtained by an optical inversion based upon the measured extinction spectrum and size distribution. Results from the present study show that the imaginary LW refractive index (k) of dust varies greatly both in magnitude and spectral shape from sample to sample, reflecting the differences in particle composition. In the 3-15 µm spectral range, k is between ˜ 0.001 and 0.92. The strength of the dust absorption at ˜ 7 and 11.4 µm depends on the amount of calcite within the samples, while the absorption between 8 and 14 µm is determined by the relative abundance of quartz and clays. The imaginary part (k) is observed to vary both from region to region and for varying sources within the same region. Conversely, for the real part (n), which is in the range 0.84-1.94, values are observed to agree for all dust samples across most of the spectrum within the error bars. This implies that while a constant n can be probably assumed for dust from different sources, a varying k should be used both at the global and the regional scale. A linear relationship between the magnitude of the imaginary refractive index at 7.0, 9.2, and 11.4 µm and the mass concentration of calcite and quartz absorbing at these wavelengths was found. We suggest that this may lead to predictive rules to estimate the LW refractive index of dust in specific bands based on an assumed or predicted mineralogical composition, or conversely, to estimate the dust composition from measurements of the LW extinction at specific wavebands. Based on the results of the present study, we recommend that climate models and remote sensing instruments operating at infrared wavelengths, such as IASI (infrared atmospheric sounder interferometer), use regionally dependent refractive indices rather than generic values. Our observations also suggest that the refractive index of dust in the LW does not change as a result of the loss of coarse particles by gravitational settling, so that constant values of n and k could be assumed close to sources and following transport. The whole dataset of the dust complex refractive indices presented in this paper is made available to the scientific community in the Supplement.

PM₁₀ and PM₂.₅ sources at an insular location in the western Mediterranean by using source apportionment techniques.

PubMed

Pey, Jorge; Alastuey, Andrés; Querol, Xavier

2013-07-01

PM₁₀ and PM₂.₅ chemical composition has been determined at a suburban insular site in the Balearic Islands (Spain) during almost one and a half year. As a result, 200 samples with more than 50 chemical parameters analyzed have been obtained. The whole database has been analyzed by two receptor modelling techniques (Principal Component Analysis and Positive Matrix Factorisation) in order to identify the main PM sources. After that, regression analyses with respect to the PM mass concentrations were conducted to quantify the daily contributions of each source. Four common sources were identified by both receptor models: secondary nitrate coupled with vehicular emissions, secondary sulphate influenced by fuel-oil combustion, aged marine aerosols and mineral dust. In addition, PCA isolated harbour emissions and a mixed anthropogenic factor containing industrial emissions; whereas PMF isolated an additional mineral factor interpreted as road dust+harbour emissions, and a vehicular abrasion products factor. The use of both methodologies appeared complementary. Nevertheless, PMF sources by themselves were better differentiated. Besides these receptor models, a specific methodology to quantify African dust was also applied. The combination of these three source apportionment tools allowed the identification of 8 sources, being 4 of them mineral (African, regional, urban and harbour dusts). As a summary, 29% of PM₁₀ was attributed to natural sources (African dust, regional dust and sea spray), whereas the proportion diminished to 11% in PM₂.₅. Furthermore, the secondary sulphate source, which accounted for about 22 and 32% of PM₁₀ and PM₂.₅, is strongly linked to the aged polluted air masses residing over the western Mediterranean in the warm period. Copyright © 2013 Elsevier B.V. All rights reserved.

Morphology and Dynamics of Jets of Comet 67P Churyumov-Gerasimenko: Early Phase Development

NASA Astrophysics Data System (ADS)

Lin, Zhong-Yi; Ip, Wing-Huen; Lai, Ian-Lin; Lee, Jui-Chi; Pajola, Maurizio; Lara, Luisa; Gutierrez, Pedro; Rodrigo, Rafael; Bodewits, Dennis; A'Hearn, Mike; Vincent, Jean-Baptiste; Agarwal, Jessica; Keller, Uwe; Mottola, Stefano; Bertini, Ivano; Lowry, Stephen; Rozek, Agata; Liao, Ying; Rosetta Osiris Coi Team

2015-04-01

The scientific camera, OSIRIS (Optical, Spectroscopic, and Infrared Remote Imaging System), onboard the Rosetta spacecraft comprises a Narrow Angle Camera (NAC) for nucleus surface and dust studies and a Wide Angle Camera (WAC) for the wide field of dust and gas coma investigations. The dynamical behavior of jets in the dust coma continuously monitored by using dust filters from the arrival at the comet (August 2014) throughout the mapping phase (Oct. 2014) is described here. The analysis will cover the study of the time variability of jets, the source regions of these jets, the excess brightness of jets relative to the averaged coma brightness, and the brightness distribution of dust jets along the projected distance. The jets detected between August and September originated mostly from the neck region (Hapi). Morphological changes appeared over a time scale of several days in September. The brightness slope of the dust jets is much steeper than the background coma. This might be related to the sublimation or fragmentation of the emitted dust grains. Inter-comparison with results from other experiments will be necessary to understand the difference between the dust emitted from Hapi and those from the head and the body of the nucleus surface. The physical properties of the Hapi jets will be compared to dust jets (and their source regions) to emerge as comet 67P moves around the perihelion.

Change in atmospheric mineral aerosols in response to climate: Last glacial period, preindustrial, modern, and doubled carbon dioxide climates

USGS Publications Warehouse

Mahowald, N.M.; Muhs, D.R.; Levis, S.; Rasch, P.J.; Yoshioka, M.; Zender, C.S.; Luo, C.

2006-01-01

Desert dust simulations generated by the National Center for Atmospheric Research's Community Climate System Model for the current climate are shown to be consistent with present day satellite and deposition data. The response of the dust cycle to last glacial maximum, preindustrial, modern, and doubled-carbon dioxide climates is analyzed. Only natural (non-land use related) dust sources are included in this simulation. Similar to some previous studies, dust production mainly responds to changes in the source areas from vegetation changes, not from winds or soil moisture changes alone. This model simulates a +92%, +33%, and -60% change in dust loading for the last glacial maximum, preindustrial, and doubled-carbon dioxide climate, respectively, when impacts of carbon dioxide fertilization on vegetation are included in the model. Terrestrial sediment records from the last glacial maximum compiled here indicate a large underestimate of deposition in continental regions, probably due to the lack of simulation of glaciogenic dust sources. In order to include the glaciogenic dust sources as a first approximation, we designate the location of these sources, and infer the size of the sources using an inversion method that best matches the available data. The inclusion of these inferred glaciogenic dust sources increases our dust flux in the last glacial maximum from 2.1 to 3.3 times current deposition. Copyright 2006 by the American Geophysical Union.

Integrated spatiotemporal characterization of dust sources and outbreaks in Central and East Asia

NASA Astrophysics Data System (ADS)

Darmenova, Kremena T.

The potential of atmospheric dust aerosols to modify the Earth's environment and climate has been recognized for some time. However, predicting the diverse impact of dust has several significant challenges. One is to quantify the complex spatial and temporal variability of dust burden in the atmosphere. Another is to quantify the fraction of dust originating from human-made sources. This thesis focuses on the spatiotemporal characterization of sources and dust outbreaks in Central and East Asia by integrating ground-based data, satellite multisensor observations, and modeling. A new regional dust modeling system capable of operating over a span of scales was developed. The modeling system consists of a dust module DuMo, which incorporates several dust emission schemes of different complexity, and the PSU/NCAR mesoscale model MM5, which offers a variety of physical parameterizations and flexible nesting capability. The modeling system was used to perform for the first time a comprehensive study of the timing, duration, and intensity of individual dust events in Central and East Asia. Determining the uncertainties caused by the choice of model physics, especially the boundary layer parameterization, and the dust production scheme was the focus of our study. Implications to assessments of the anthropogenic dust fraction in these regions were also addressed. Focusing on Spring 2001, an analysis of routine surface meteorological observations and satellite multi-sensor data was carried out in conjunction with modeling to determine the extent to which integrated data set can be used to characterize the spatiotemporal distribution of dust plumes at a range of temporal scales, addressing the active dust sources in China and Mongolia, mid-range transport and trans-Pacific, long-range transport of dust outbreaks on a case-by-case basis. This work demonstrates that adequate and consistent characterization of individual dust events is central to establishing a reliable climatology, ultimately leading to improved assessments of dust impacts on the environment and climate. This will also help to identify the appropriate temporal and spatial scales for adequate intercomparison between model results and observational data as well as for developing an integrated analysis methodology for dust studies.

Climate Change Implications and Use of Early Warning Systems for Global Dust Storms

NASA Astrophysics Data System (ADS)

Harriman, L.

2014-12-01

Increased changes in land cover and global climate have led to increased frequency and/or intensity of dust storms in some regions of the world. Early detection and warning of dust storms, in conjunction with effective and widespread information broadcasts, will be essential to the prevention and mitigation of future risks and impacts to people and the environment. Since frequency and intensity of dust storms can vary from region to region, there is a demonstrated need for more research to be conducted over longer periods of time to analyze trends of dust storm events [1]. Dust storms impact their origin area, but also land, water and people a great distance away from where dust finally settles [2, 3]. These transboundary movements and accompanying impacts further warrant the need for global collaboration to help predict the onset, duration and path of a dust storm. Early warning systems can help communicate when a dust storm is occurring, the projected intensity of the dust storm and its anticipated physical impact over a particular geographic area. Development of regional dust storm models, such as CUACE/Dust for East Asia, and monitoring networks, like the Sand and Dust Storm Warning Network operated by the World Meteorological Organization, and the use of remote sensing and satellite imagery derived products [4], including MODIS, are currently being incorporated into early warning and monitoring initiatives. However, to increase future certainty of impacts of dust storms on vulnerable populations and ecosystems, more research is needed to analyze the influences of human activities, seasonal variations and long-term climatic patterns on dust storm generation, movement and impact. Sources: [1] Goudie, A.S. (2009), Dust storms: recent developments, J Environ. Manage., 90. [2] Lee, H., and Liu, C. (2004), Coping with dust storm events: information, impacts, and policymaking in Taiwan, TAO, 15(5). [3] Marx, S.K., McGowan, H.A., and Balz, K.S. (2009), Long-range dust transport from eastern Australia: a proxy for Holocene aridity and ENSO-type climate variability, Earth Planet Sci. Lett., 282. [4] Kimura, R. (2012), Factors contributing to dust storms in source regions producing the yellow-sand phenomena observed in Japan from 1993 to 2002, J. Arid Environ. 80

Effective and Accurate Morphology Models for Asian and Saharan Mineral Dust Scattering Properties

NASA Astrophysics Data System (ADS)

Stegmann, P.; Yang, P.

2017-12-01

It is well known that mineral dust particles from desert sources can have a significant influence on the planetary radiation balance. In order to determine the sign and magnitude of the dust radiative forcing effect, complex models have been and continue to be developed. Key factors which influence the single-scattering properties of mineral dust are dust source regions and thus mineralogical composition, and its mixture with water, sea salt, and products of human activity, such as soot. The ensemble of mineral dust scattering particles may then be modeled either as a simple placeholder shape, often ellipsoidal, through the utilization of an appropriate effective medium refractive index scheme. On the other hand, the scattering particles may be represented in a more rigorous manner, such as Voronoi-tessellated aggregates including fractal soot chains. The consequences and differences of either choice are investigated in the project at hand. It will be shown that the effective medium model indicates a drastic dependence of the mineral dust particle composition on the particle size. Thus the refractive index of a dust particle is in fact a function of its size, amongst other factors. Regional differences between African and Asian mineral dust are also of significance.

How Early Holocene Greening of the Afro-Asian Dust Belt Changed Sources of Mineral Dust in West Asia

NASA Astrophysics Data System (ADS)

Pourmand, A.; Sharifi, A.; Goes, L. M.; Clement, A. C.; Canuel, E. A.; Naderi Beni, A.; Ahmady-Birgani, H.

2016-12-01

Production, transport and deposition of mineral dust have significant temporal and spatial impacts on different components of the Earth systems. In modern times, dust plumes can be associated with their source origin(s) using satellite and land-based measurements and back-trajectory reconstruction of air masses. Reconstructing past changes in the sources of mineral dust as related to changes in climate, however, must rely on the knowledge of the geochemical and mineralogical composition of modern and paleo-dust, and their potential source origins. In this contribution, we present a 13,000-year record of variations in radiogenic Sr-Nd-Hf isotopes and Rare Earth Element (REE) anomalies from an ombrotrophic (rain fed) peat core in NW Iran as proxies of past changes in sources of dust over West Asia. The geochemical fingerprint of dust particles deposited during the low-flux, early Holocene period (11,700-6,000 yr BP) is distinctly different from times of high dust fluxes during the Younger Dryas, and that of the mid-late Holocene. This indicates that the composition of mineral dust deposited at the receptor site changed as a function of prevailing atmospheric circulation regimes and land exposure. Simulations of atmospheric circulation over the region show the Northern Hemisphere Westerly Jet (NHWJ) was displaced poleward across the study area during the early Holocene when solar insolation was higher. This shift, coupled with lower dust emissions simulated based on greening of the Afro-Asian Dust Belt during the early Holocene likely led to potential sources in Central Asia to dominate dust export to West Asia during this period, in contrast to the dominant western and southwest Asian and Eastern African sources that prevail during the modern period.

Geochemical and mineralogical evidence for Sahara and Sahel dust additions to Quaternary soils on Lanzarote, eastern Canary Islands, Spain

USGS Publications Warehouse

Muhs, D.R.; Budahn, J.; Skipp, G.; Prospero, J.M.; Patterson, D.; Bettis, E. Arthur

2010-01-01

Africa is the most important source of dust in the world today, and dust storms are frequent on the nearby Canary Islands. Previous workers have inferred that the Sahara is the most important source of dust to Canary Islands soils, with little contribution from the Sahel region. Soils overlying a late Quaternary basalt flow on Lanzarote, Canary Islands, contain, in addition to volcanic minerals, quartz and mica, exotic to the island's bedrock. Kaolinite in the soils also likely has an exotic origin. Trace-element geochemistry shows that the soils are derived from varying proportions of locally derived basalt and African dust. Major-element geochemistry, clay mineralogy and interpretation of satellite imagery suggest that dust additions to the Canary Islands come not only from the Sahara Desert, but also from the Sahel region. ?? Published 2010. This article is a US Government work and is in the public domain in the USA.

Transport of Aerosols: Regional and Global Implications for Climate, Weather, and Air Quality

NASA Technical Reports Server (NTRS)

Chin, Mian; Diehl, Thomas; Yu, Hongbin; Bian, Huisheng; Remer, Lorraine; Kahn, Ralph

2008-01-01

Long-range transport of atmospheric aerosols can have a significant impact on global climate, regional weather, and local air quality. In this study, we use a global model GOCART together with satellite data and ground-based measurements to assess the emission and transport of pollution, dust, biomass burning, and volcanic aerosols and their implications. In particular, we will show the impact of emissions and long-range transport of aerosols from major pollution and dust source regions to (1) the surface air quality, (2) the atmospheric heating rates, and (3) surface radiation change near the source and downwind regions.

Global View of Aerosol Vertical Distributions from CALIPSO Lidar Measurements and GOCART Simulations: Regional and Seasonal Variations

NASA Technical Reports Server (NTRS)

Yu, Hongbin; Chin, Mian; Winker, David M.; Omar, Ali H.; Liu, Zhaoyan; Kittaka, Chieko; Diehl, Thomas

2010-01-01

This study examines seasonal variations of the vertical distribution of aerosols through a statistical analysis of the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) lidar observations from June 2006 to November 2007. A data-screening scheme is developed to attain good quality data in cloud-free conditions, and the polarization measurement is used to separate dust from non-dust aerosol. The CALIPSO aerosol observations are compared with aerosol simulations from the Goddard Chemistry Aerosol Radiation Transport (GOCART) model and aerosol optical depth (AOD) measurements from the MODerate resolution Imaging Spectroradiometer (MODIS). The CALIPSO observations of geographical patterns and seasonal variations of AOD are generally consistent with GOCART simulations and MODIS retrievals especially near source regions, while the magnitude of AOD shows large discrepancies in most regions. Both the CALIPSO observation and GOCART model show that the aerosol extinction scale heights in major dust and smoke source regions are generally higher than that in industrial pollution source regions. The CALIPSO aerosol lidar ratio also generally agrees with GOCART model within 30% on regional scales. Major differences between satellite observations and GOCART model are identified, including (1) an underestimate of aerosol extinction by GOCART over the Indian sub-continent, (2) much larger aerosol extinction calculated by GOCART than observed by CALIPSO in dust source regions, (3) much weaker in magnitude and more concentrated aerosol in the lower atmosphere in CALIPSO observation than GOCART model over transported areas in midlatitudes, and (4) consistently lower aerosol scale height by CALIPSO observation than GOCART model. Possible factors contributing to these differences are discussed.

Meteorological Situations Favouring the Development of Dust Plumes over Iceland

NASA Astrophysics Data System (ADS)

Schepanski, K.; Szodry, K.

2017-12-01

The knowledge on mineral dust emitted at high latitudes is limited, but its impact on the polar environments is divers. Within a warming climate, dust emitted from regions in cold climates is expected to increase due to the retreat of the ice sheet and increasing melting rates. Therefore, and for its extensive impacts on different aspects of the climate system, a better understanding of the atmospheric dust life-cycle at high latitudes/cold climates in general, and the spatio-temporal distribution of dust sources in particular, are essential. At high-latitudes, glacio-fluvial sediments as found on river flood plains e.g. supplied by glaciers are prone to wind erosion when dry and bare. In case of the occurrence of strong winds, sediments are blown out and dust plumes develop. As dust uplift is controlled by soil surface characteristics, the availability of suitable sediments, and atmospheric conditions, an interannual variability in dust source activity is expected. We investigated atmospheric circulation patterns that favour the development of dust plumes over Iceland, which presents a well-known dust source at high latitudes. Using the atmosphere model COSMO (COnsortium for Small-scale MOdeling), we analysed the wind speed distribution over the Iceland region for identified and documented dust cases. As one outcome of the study, the position of the Icelandic low, the anticyclones located over Northern Europe, and the resulting pressure gradients are of particular relevance. The interaction of the synoptic-scale winds with the Icelandic orography may locally enhance the wind speeds and thus foster local dust emission. Results from this study suggest that the atmospheric circulation determined by the pressure pattern is of particular relevance for the formation of dust plumes entering the North Atlantic.

Laboratory estimate of the regional shortwave refractive index and single scattering albedo of mineral dust from major sources worldwide

NASA Astrophysics Data System (ADS)

Di Biagio, C.; Formenti, P.; Caponi, L.; Cazaunau, M.; Pangui, E.; Journet, E.; Nowak, S.; Caquineau, S.; Andreae, M. O.; Kandler, K.; Saeed, T.; Piketh, S.; Seibert, D.; Williams, E.; Balkanski, Y.; Doussin, J. F.

2017-12-01

Mineral dust is one of the most abundant aerosol species in the atmosphere and strongly contributes to the global and regional direct radiative effect. Still large uncertainties persist on the magnitude and overall sign of the dust direct effect, where indeed one of the main unknowns is how much mineral dust absorbs light in the shortwave (SW) spectral range. Aerosol absorption is represented both by the imaginary part (k) of the complex refractive index or the single scattering albedo (SSA, i.e. the ratio of the scattering to extinction coefficient). In this study we present a new dataset of SW complex refractive indices and SSA for mineral dust aerosols obtained from in situ measurements in the 4.2 m3 CESAM simulation chamber at LISA (Laboratoire Interuniversitaire des Systemes Atmospheriques) in Créteil, France. Investigated dust aerosol samples were issued from major desert sources worldwide, including the African Sahara and Sahel, Eastern Asia, the Middle East, Southern Africa, Australia, and the Americas, with differing iron oxides content. Results from the present study provide a regional mapping of the SW absorption by dust and show that the imaginary part of the refractive index largely varies (by up to a factor 6, 0.003-0.02 at 370 nm and 0.001-0.003 at 950 nm) for the different source areas due to the change in the particle iron oxide content. The SSA for dust varies between 0.75-0.90 at 370 nm and 0.95-0.99 at 950 nm, with the largest absorption observed for Sahelian and Australian dust aerosols. Our range of variability for k and SSA is well bracketed by already published literature estimates, but suggests that regional‒dependent values should be used in models. The possible relationship between k and the dust iron oxides content is investigated with the aim of providing a parameterization of the regional‒dependent dust absorption to include in climate models.

Asian dust transportation and fertilizing the coastal and open ocean in the Northern Pacific (Invited)

NASA Astrophysics Data System (ADS)

Gao, H.; Xiaohong Yao, Jinhui Shi, Jianhua Qi

2010-12-01

Dust storm carries a large amount of aerosol particles, sweeps continents and exports to oceans. When these aerosol particles deposit in ocean, which provides abundant nutrients such as nitrogen and iron for ocean ecosystem, increases the primary production and induces algae bloom. Asian dust storm generates at a high latitude and a high elevation and is obvious a hemispheric scale phenomenon. Dust sources in East Asia are one of the major dust sources on the earth which contribute to 5%-40% of the global dust release. The regions affected by the Asian dust storm include not only China and Mongolia but also the downwind Korea, Japan, the Pacific Ocean, the west coast of America, even the subarctic region and Europe. The Asian dust storm is obviously a hemispheric scale phenomenon, which has more important impact on the ecosystem in the western Pacific. Asian dust is unique not only in morphology, soil texture, and dust storm activities, but also mixing and capturing anthropogenic air pollutants on the transport pathway. Deposition of Asian dust substantially affects surface biological productivity. To improve understandings of Asian dust and its effect on ocean ecosystem from the coastal sea to open ocean, ADOES (Asian Dust and Ocean EcoSystem) was proposed under the frame of international SOLAS (Surface Ocean-Lower Atmosphere Study). A series of studies were performed in high- nutrient low-chlorophyll (HNLC), low-nutrient low-chlorophyll (LNLC) and eutrophication coastal regions of the Pacific Ocean. These studies provided evidence of biotic response to natural iron fertilization caused by Asian dust particles in the subarctic North Pacific and showed that dust storm episodes were significant in the initiation of spring blooms in the East China Sea. On-board incubations on the cruise in a LNLC region of the western Pacific at the southeast of Japan showed different responses of ocean ecosystem to nitrogen and dust fertilization. Correlation of the Asian dust storms with chlorophyll, primary productivity and algae blooms in the coastal seas of China from 1998 to 2008 were also illustrated.

Aerosol Absorption by Black Carbon and Dust: Implications of Climate Change and Air Quality in Asia

NASA Technical Reports Server (NTRS)

Chin, Mian

2010-01-01

Atmospheric aerosol distributions from 2000 to 2007 are simulated with the global model GOCART to attribute light absorption by aerosol to its composition and sources. We show the seasonal and interannual variations of absorbing aerosols in the atmosphere over Asia, mainly black carbon and dust. and their linkage to the changes of anthropogenic and dust emissions in the region. We compare our results with observations from satellite and ground-based networks, and estimate the importance of black carbon and dust on regional climate forcing and air quality.

Identifying Dust Sources by Positive Matrix Factorization (PMF)

NASA Astrophysics Data System (ADS)

Engelbrecht, Johann P.

2010-05-01

This presentation is on the source attribution by Positive Matrix Factorization (PMF) of aerosol samples collected in Iraq, a major source of mineral dust in the Middle East. Globally transported mineral dust from North Africa, the Middle East, China, and elsewhere are routinely being sampled at high elevation monitoring sites such as those on the Canary Islands and Hawaii, and many ambient monitoring sites worldwide. Chemical results of these filter samples reflect differences in sources impacting at each site, further complicated by the regional geomorphology and meteorology. Trace elements, isotopes, elemental ratios, and mineralogy are generally being used to pinpoint geological source regions of natural and anthropogenic dusts. A receptor site is seldom impacted by only one source at a time. Dust palls are continually being modified by added dust from soils across which they migrate, also by particle segregation in the dust plume, and precipitation of the coarser particles. The result is that dust is a mixture, with contributions from different sources, each with a different chemical and mineralogical signature. PMF is a non-negative factorization procedure that produces only positive factor scores and loadings, in contrast to classical factor analysis (FA) and Principal Components Analysis (PCA). PMF enables us to resolve factors (chemical signatures) for source types contributing to the ambient chemical data set, and also models the source-type contributions to individual ambient samples. The latter can often be related to specific source regions. PMF was applied separately to two ambient data sets collected in Iraq in 2006, the one on Teflon membrane filters and the other on quartz fiber. Each of the filter types were previously analyzed for different chemical species: Teflon membrane for elements, by XRF and ICP-MS, while quartz fiber filters were analyzed for ions and carbon. [Engelbrecht et al. 2009] A set of 392 Teflon filter samples analyzed for 25 elemental species was modeled by PMF. A five factor solution identified three soil factors, a silicate soil, limestone soil, and a gypsum soil, as well as a salt factor and an anthropogenic metal factor. Similarly, a set of 362 quartz filter samples analyzed for 10 selected chemical species was modeled by PMF. A five factor solution provided a limestone-gypsum soil, diesel combustion, secondary ammonium sulfate, salt and agricultural-burnpit combustion source type. Examples of time series plots of PMF factor contributions for each of six sampling sites (Balad, Baghdad, Tallil, Tikrit, Taji, and Al Asad) will be discussed. Engelbrecht , J. P., McDonald, E. V., Gillies, J. A., Jayanty, R. K. M., Casuccio, G., and Gertler, A. W., 2009, Characterizing mineral dusts and other aerosols from the Middle East - Part 1: Ambient sampling: Inhalation Toxicology, v. 21, p. 297-326.

Geochemical characterization of critical dust source regions in the American West

NASA Astrophysics Data System (ADS)

Aarons, Sarah M.; Blakowski, Molly A.; Aciego, Sarah M.; Stevenson, Emily I.; Sims, Kenneth W. W.; Scott, Sean R.; Aarons, Charles

2017-10-01

The generation, transport, and deposition of mineral dust are detectable in paleoclimate records from land, ocean, and ice, providing valuable insight into earth surface conditions and cycles on a range of timescales. Dust deposited in marine and terrestrial ecosystems can provide critical nutrients to nutrient-limited ecosystems, and variations in dust provenance can indicate changes in dust production, sources and transport pathways as a function of climate variability and land use change. Thus, temporal changes in locations of dust source areas and transport pathways have implications for understanding interactions between mineral dust, global climate, and biogeochemical cycles. This work characterizes dust from areas in the American West known for dust events and/or affected by increasing human settlement and livestock grazing during the last 150 years. Dust generation and uplift from these dust source areas depends on climate and land use practices, and the relative contribution of dust has likely changed since the expansion of industrialization and agriculture into the western United States. We present elemental and isotopic analysis of 28 potential dust source area samples analyzed using Thermal Ionization Mass Spectrometry (TIMS) for 87Sr/86Sr and 143Nd/144Nd composition and Multi-Collector Inductively Coupled Plasma Mass Spectrometer (MC-ICPMS) for 176Hf/177Hf composition, and ICPMS for major and trace element concentrations. We find significant variability in the Sr, Nd, and Hf isotope compositions of potential source areas of dust throughout western North America, ranging from 87Sr/86Sr = 0.703699 to 0.740236, εNd = -26.6 to 2.4, and εHf = -21.7 to -0.1. We also report differences in the trace metal and phosphorus concentrations in the geologic provinces sampled. This research provides an important resource for the geochemical tracing of dust sources and sinks in western North America, and will aid in modeling the biogeochemical impacts of increased dust generation and deposition caused by higher drought frequency and human activity.

ON THE ORIGIN OF INNER COMA STRUCTURES OBSERVED BY ROSETTA DURING A DIURNAL ROTATION OF COMET 67P/CHURYUMOV–GERASIMENKO

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kramer, Tobias; Noack, Matthias

2016-05-20

The Rosetta probe around comet 67P/Churyumov–Gerasimenko (67P) reveals an anisotropic dust distribution of the inner coma with jet-like structures. The physical processes leading to jet formation are under debate, with most models for cometary activity focusing on localized emission sources, such as cliffs or terraced regions. Here we suggest, by correlating high-resolution simulations of the dust environment around 67P with observations, that the anisotropy and the background dust density of 67P originate from dust released across the entire sunlit surface of the nucleus rather than from few isolated sources. We trace back trajectories from coma regions with high local dustmore » density in space to the non-spherical nucleus and identify two mechanisms of jet formation: areas with local concavity in either two dimensions or only one. Pits and craters are examples of the first case; the neck region of the bi-lobed nucleus of 67P is an example of the latter case. The conjunction of multiple sources, in addition to dust released from all other sunlit areas, results in a high correlation coefficient (∼0.8) of the predictions with observations during a complete diurnal rotation period of 67P.« less

Palaeo-dust records: A window to understanding past environments

NASA Astrophysics Data System (ADS)

Marx, Samuel K.; Kamber, Balz S.; McGowan, Hamish A.; Petherick, Lynda M.; McTainsh, Grant H.; Stromsoe, Nicola; Hooper, James N.; May, Jan-Hendrik

2018-06-01

Dust entrainment, transport over vast distances and subsequent deposition is a fundamental part of the Earth system. Yet the role and importance of dust has been underappreciated, due largely to challenges associated with recognising dust in the landscape and interpreting its depositional history. Despite these challenges, interest in dust is growing. Technical advances in remote sensing and modelling have improved understanding of dust sources and production, while advances in sedimentology, mineralogy and geochemistry (in particular) have allowed dust to be more easily distinguished within sedimentary deposits. This has facilitated the reconstruction of records of dust emissions through time. A key advance in our understanding of dust has occurred following the development of methods to geochemically provenance (fingerprint) dust to its source region. This ability has provided new information on dust transport pathways, as well as the reach and impact of dust. It has also expanded our understanding of the processes driving dust emissions over decadal to millennial timescales through linking dust deposits directly to source area conditions. Dust provenance studies have shown that dust emission, transport and deposition are highly sensitive to variability in climate. They also imply that dust emissions are not simply a function of the degree of aridity in source areas, but respond to a more complex array of conditions, including sediment availability. As well as recording natural variability, dust records are also shown to sensitively track the impact of human activity. This is reflected by both changing dust emission rates and changing dust chemistry. Specific examples of how dust responds to, and records change, are provided with our work on dust emissions from Australia, the most arid inhabited continent and the largest dust source in the Southern Hemisphere. These case studies show that Australian dust emissions reflect hydro-climate variability, with reorganisation of Australian dust source areas occurring during the mid to late Holocene. Dust emissions are shown to sensitively map the structure of the Last Glacial Maximum in Australia, demonstrating that this period was associated with enhanced, but also variable dust emissions, driven by changing sources area conditions. Finally we show how dust emissions have responded to the arrival of Europeans and the associated onset of broad-scale agriculture across the Australian continent.

Persistent organic contaminants in Saharan dust air masses in West Africa, Cape Verde and the eastern Caribbean

USGS Publications Warehouse

Garrison, Virginia H.; Majewski, Michael S.; Foreman, William T.; Genualdi, Susan A.; Mohammed, Azad; Massey Simonich, Stacy L.

2014-01-01

Anthropogenic semivolatile organic compounds (SOCs) that persist in the environment, bioaccumulate, are toxic at low concentrations, and undergo long-range atmospheric transport (LRT) were identified and quantified in the atmosphere of a Saharan dust source region (Mali) and during Saharan dust incursions at downwind sites in the eastern Caribbean (U.S. Virgin Islands, Trinidad and Tobago) and Cape Verde. More organochlorine and organophosphate pesticides (OCPPs), polycyclic aromatic hydrocarbons (PAHs), and polychlorinated biphenyl (PCB) congeners were detected in the Saharan dust region than at downwind sites. Seven of the 13 OCPPs detected occurred at all sites: chlordanes, chlorpyrifos, dacthal, dieldrin, endosulfans, hexachlorobenzene (HCB), and trifluralin. Total SOCs ranged from 1.9–126 ng/m3 (mean = 25 ± 34) at source and 0.05–0.71 ng/m3 (mean = 0.24 ± 0.18) at downwind sites during dust conditions. Most SOC concentrations were 1–3 orders of magnitude higher in source than downwind sites. A Saharan source was confirmed for sampled air masses at downwind sites based on dust particle elemental composition and rare earth ratios, atmospheric back trajectory models, and field observations. SOC concentrations were considerably below existing occupational and/or regulatory limits; however, few regulatory limits exist for these persistent organic compounds. Long-term effects of chronic exposure to low concentrations of SOCs are unknown, as are possible additive or synergistic effects of mixtures of SOCs, biologically active trace metals, and mineral dust particles transported together in Saharan dust air masses.

The modern atmospheric background dust load: Recognition in Central Asian snowpack, and compositional constraints

USGS Publications Warehouse

Hinkley, T.; Pertsiger, F.; Zavjalova, L.

1997-01-01

Dusts in strata of snowpack in the Alai-Pamir range, Kirghizstan, Central Asia, have chemical compositions that are in the same restricted range as those of the dusts found in snowpacks at three other locations: central south Greenland, the St. Elias range (Alaska), and coastal Antarctica, where special-type local dust sources certainly cannot dominate. This similarity at the four widely separated sites appears to indicate that there is a modern atmospheric background dust that is the same on a regional, hemispheric, or global scale. The common compositional range is that of average crustal rock, or of moderately ferromagnesian volcanic rock. It is not that of carbonate, nor highly siliciceous rocks. Previously, the existence of an atmospheric background dust has been postulated only on the basis of its particle size distribution, and only from observations in polar regions. The present study partially determines the chemical composition of the background dust, and confirms its existence in snowpack at four localities worldwide, including the center of the earth's largest continent where dusts of local source have considerable influence. U.S. copyright. Published in 1997 by the American Geophysical Union.

Can land use intensification in the Mallee, Australia increase the supply of soluble iron to the Southern Ocean?

PubMed Central

Bhattachan, Abinash; D'Odorico, Paolo

2014-01-01

The supply of soluble iron through atmospheric dust deposition limits the productivity of the Southern Ocean. In comparison to the Northern Hemisphere, the Southern Hemisphere exhibits low levels of dust activity. However, given their proximity to the Southern Ocean, dust emissions from continental sources in the Southern Hemisphere could have disproportionate impact on ocean productivity. Australia is the largest source of dust in the Southern Hemisphere and aeolian transport of dust has major ecological, economic and health implications. In the Mallee, agriculture is a major driver of dust emissions and dust storms that affect Southeastern Australia. In this study, we assess the dust generating potential of the sediment from the Mallee, analyze the sediment for soluble iron content and determine the likely depositional region of the emitted dust. Our results suggest that the Mallee sediments have comparable dust generating potential to other currently active dust sources in the Southern Hemisphere and the dust-sized fraction is rich in soluble iron. Forward trajectory analyses show that this dust will impact the Tasman Sea and the Australian section of the Southern Ocean. This iron-rich dust could stimulate ocean productivity in future as more areas are reactivated as a result of land-use and droughts. PMID:25109703

Polybrominated Diphenyl Ethers in Residential Dust: Sources of Variability

PubMed Central

Whitehead, Todd P.; Brown, F. Reber; Metayer, Catherine; Park, June-Soo; Does, Monique; Petreas, Myrto X.; Buffler, Patricia A.; Rappaport, Stephen M.

2013-01-01

We characterized the sources of variability for polybrominated diphenyl ethers (PBDEs) in residential dust and provided guidance for investigators who plan to use residential dust to assess exposure to PBDEs. We collected repeat dust samples from 292 households in the Northern California Childhood Leukemia Study during two sampling rounds (from 2001–2007 and during 2010) using household vacuum cleaners and measured 22 PBDEs using high resolution gas chromatography-high resolution mass spectrometry. Median concentrations for individual PBDEs ranged from <0.1–2,500 ng per g of dust. For each of eight representative PBDEs, we used a random-effects model to apportion total variance into regional variability (0–11%), intra-regional between-household variability (17–50%), within-household variability over time (38–74%), and within-sample variability (0–23%) and we used a mixed-effects model to identify determinants of PBDE levels. Regional differences in PBDE dust levels were associated with residential characteristics that differed by region, including the presence of furniture with exposed or crumbling foam and the recent installation of carpets in the residence. Intra-regional differences between households were associated with neighborhood urban density, racial and ethnic characteristics, and to a lesser extent, income. For some PBDEs, a decreasing time trend explained a modest fraction of the within-household variability; however, most of the within-household variability was unaccounted for by our mixed-effects models. Our findings indicate that it may be feasible to use residential dust for retrospective assessment of PBDE exposures in studies of children’s health (e.g., the Northern California Childhood Leukemia Study). PMID:23628589

Aerosol transport over the western Mediterranean basin: Evidence of the contribution of fine particles to desert dust plumes over Alborán Island

NASA Astrophysics Data System (ADS)

Valenzuela, A.; Olmo, F. J.; Lyamani, H.; Granados-Muñoz, M. J.; Antón, M.; Guerrero-Rascado, J. L.; Quirantes, A.; Toledano, C.; Perez-Ramírez, D.; Alados-Arboledas, L.

2014-12-01

Eight months (June 2011 to January 2012) of aerosol property data were obtained at the remote site of Alborán Island (35.95°N, 3.03°W) in the western Mediterranean basin. The aim of this work is to assess the aerosol properties according to air mass origin and transport over this remote station with a special focus on air mass transport from North Africa. For air masses coming from North Africa, different aerosol properties showed strong contributions from mineral dust lifted from desert areas. Nevertheless, during these desert dust intrusions, some atmospheric aerosol properties are clearly different from pure mineral dust particles. Thus, Angström exponent α(440-870) presents larger values than those reported for pure desert dust measured close to dust source regions. These results combine with α(440, 670) - α(670, 870) ≥ 0.1 and low single scattering albedo (ω(λ)) values, especially at the largest wavelengths. Most of the desert dust intrusions over Alborán can be described as a mixture of dust and anthropogenic particles. The analyses support that our results apply to North Africa desert dust air masses transported from different source areas. Therefore, our results indicate a significant contribution of fine absorbing particles during desert dust intrusions over Alborán arriving from different source regions. The aerosol optical depth data retrieved from Sun photometer measurements have been used to check Moderate Resolution Imaging Spectroradiometer retrievals, and they show reasonable agreement, especially for North African air masses.

Enhancing weak transient signals in SEVIRI false color imagery: Application to dust source detection in southern Africa

NASA Astrophysics Data System (ADS)

Murray, J. E.; Brindley, H. E.; Bryant, R. G.; Russell, J. E.; Jenkins, K. F.; Washington, R.

2016-09-01

A method is described to significantly enhance the signature of dust events using observations from the Spinning Enhanced Visible and InfraRed Imager (SEVIRI). The approach involves the derivation of a composite clear-sky signal for selected channels on an individual time step and pixel basis. These composite signals are subtracted from each observation in the relevant channels to enhance weak transient signals associated with either (a) low levels of dust emission or (b) dust emissions with high salt or low quartz content. Different channel combinations, of the differenced data from the steps above, are then rendered in false color imagery for the purpose of improved identification of dust source locations and activity. We have applied this clear-sky difference (CSD) algorithm over three (globally significant) source regions in southern Africa: the Makgadikgadi Basin, Etosha Pan, and the Namibian and western South African coast. Case study analyses indicate three notable advantages associated with the CSD approach over established image rendering methods: (i) an improved ability to detect dust plumes, (ii) the observation of source activation earlier in the diurnal cycle, and (iii) an improved ability to resolve and pinpoint dust plume source locations.

Aeolian system dynamics derived from thermal infrared data

NASA Astrophysics Data System (ADS)

Scheidt, Stephen Paul

Thermal infrared (TIR) remote-sensing and field-based observations were used to study aeolian systems, specifically sand transport pathways, dust emission sources and Saharan atmospheric dust. A method was developed for generating seamless and radiometrically accurate mosaics of thermal infrared data from the Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) instrument. Using a combination of high resolution thermal emission spectroscopy results of sand samples and mosaic satellite data, surface emissivity was derived to map surface composition, which led to improvement in the understanding of sand accumulation in the Gran Desierto of northern Sonora, Mexico. These methods were also used to map sand transport pathways in the Sahara Desert, where the interaction between sand saltation and dust emission sources was explored. The characteristics and dynamics of dust sources were studied at White Sands, NM and in the Sahara Desert. At White Sands, an application was developed for studying the response of dust sources to surface soil moisture based on the relationship between soil moisture, apparent thermal inertia and the erosion potential of dust sources. The dynamics of dust sources and the interaction with sand transport pathways were also studied, focusing on the Bodele Depression of Chad and large dust sources in Mali and Mauritania. A dust detection algorithm was developed using ASTER data, and the spectral emissivity of observed atmospheric dust was related to the dust source area in the Sahara. At the Atmospheric Observatory (IZO) in Tenerife, Spain where direct measurement of the Saharan Air Layer could be made, the cycle of dust events occurring in July 2009 were examined. From the observation tower at the IZO, measurements of emitted longwave atmospheric radiance in the TIR wavelength region were made using a Forward Looking Infrared Radiometer (FLIR) handheld camera. The use of the FLIR to study atmospheric dust from the Saharan is a new application. Supporting data from AERONET and other orbital data enabled study of net radiative forcing.

Derivation of an observation-based map of North African dust emission

DOE Office of Scientific and Technical Information (OSTI.GOV)

Evan, Amato T.; Fiedler, Stephanie; Zhao, Chun

Changes in the emission, transport and deposition of aeolian dust have profound effects on regional climate, so that characterizing the lifecycle of dust in observations and improving the representation of dust in global climate models is necessary. A fundamental aspect of characterizing the dust cycle is quantifying surface dust fluxes, yet no spatially explicit estimates of this flux exist for the World’s major source regions. Here we present a novel technique for creating a map of the annual mean emitted dust flux for North Africa based on retrievals of dust storm frequency from the Meteosat Second Generation Spinning Enhanced Visiblemore » and InfraRed Imager (SEVIRI) and the relationship between dust storm frequency and emitted mass flux derived from the output of five models that simulate dust. Our results suggest that 64 (±16)% of all dust emitted from North Africa is from the Bodélé depression, and that 13 (±3)% of the North African dust flux is from a depression lying in the lee of the Aïr and Hoggar Mountains, making this area the second most important region of emission within North Africa.« less

PERSPECTIVE: Dust, fertilization and sources

NASA Astrophysics Data System (ADS)

Remer, Lorraine A.

2006-11-01

Aerosols, tiny suspended particles in the atmosphere, play an important role in modifying the Earth's energy balance and are essential for the formation of cloud droplets. Suspended dust particles lifted from the world's arid regions by strong winds contain essential minerals that can be transported great distances and deposited into the ocean or on other continents where productivity is limited by lack of usable minerals [1]. Dust can transport pathogens as well as minerals great distance, contributing to the spread of human and agricultural diseases, and a portion of dust can be attributed to human activity suggesting that dust radiative effects should be included in estimates of anthropogenic climate forcing. The greenish and brownish tints in figure 1 show the wide extent of monthly mean mineral dust transport, as viewed by the MODerate resolution Imaging Spectroradiometer (MODIS) satellite sensor. The monthly mean global aerosol system for February 2006 from the MODIS aboard the Terra satellite Figure 1. The monthly mean global aerosol system for February 2006 from the MODIS aboard the Terra satellite. The brighter the color, the greater the aerosol loading. Red and reddish tints indicate aerosol dominated by small particles created primarily from combustion processes. Green and brownish tints indicate larger particles created from wind-driven processes, usually transported desert dust. Note the bright green band at the southern edge of the Saharan desert, the reddish band it must cross if transported to the southwest and the long brownish transport path as it crosses the Atlantic to South America. Image courtesy of the NASA Earth Observatory (http://earthobservatory.nasa.gov). Even though qualitatively we recognize the extent and importance of dust transport and the role that it plays in fertilizing nutrient-limited regions, there is much that is still unknown. We are just now beginning to quantify the amount of dust that exits one continental region and the fraction that arrives at another continent [2]. At the deposition end of the chain, it is still unclear how the limited minerals in the dust such as iron are released for uptake by organisms either on land or in the ocean. Not all dust deposited into oceans results in a phytoplankton bloom. The process requires a chemical pathway that mobilizes a fraction of the iron into soluble form. Meskhidze et al [3] show that phytoplankton blooms following dust transport from the Gobi desert in Asia into the Pacific ocean result in a phytoplankton bloom only if the dust is accompanied by high initial SO2-to-dust ratios, suggesting that sulfuric acid coatings on the dust particle mobilize the embedded iron in the dust for phytoplankton uptake. Quantifying transport, deposition and nutrient availability are the latter ends of a puzzle that must begin by identifying and quantifying dust emission at the sources. The emission process is complex at the microscale requiring the right conditions for saltation and bombardment, which makes identification and inclusion of sources in global transport models very difficult. The result is that estimates of annual global dust emissions range from 1000 to 3000 Tg per year [4]. Even as global estimates of dust emissions are uncertain, localizing the sources brings even greater uncertainty. It has been recognized for several years that dust sources are not uniformly distributed over the arid regions of the Earth, but are regulated to topographic lows associated with dried lake deposits [5]. Using aerosol information from satellites, a comprehensive map of the world's source regions shows sources localized to specific areas of the Earth's arid regions [6]. Still these maps suggest broad emission sources covering several degrees of latitude and longitude. In the paper by Koren and co-authors [7] appearing in this issue, one particular dust source, the Bodélé depression in Chad, is analyzed in detail. They find that the specific topography of the depression combined with the prevailing wind direction in the winter provides perfect conditions for aerosol saltation, uplift and transport. The winter Bodélé dust is carried over the populated regions of west Africa where it can be affected by smoke and urban pollution before it continues transport over the Atlantic and towards Amazonia. Although Koren et al do not speculate on the chemical possibilities in their paper, the interaction between the dust and the pollutants provides opportunity for acids to coat the dust particles and to mobilize the iron compounds, creating a highly efficient fertilizing agent for ocean phytoplankton and the biota of the Amazon forest. Koren et al do quantify the dust emission of the Bodélé depression, estimating that this small area produces approximately 50% of the Saharan dust deposited in the Amazon. The findings of Koren and his co-authors suggest that dust emission sources may be highly localized spots in the Earth's deserts that can be mapped precisely by satellites of moderate to fine resolution. Like fire hot spots that localize smoke emission, desert dust hot spots can be identified with great detail. This can provide aerosol transport models with better source emission information and improve estimates that will help in making estimates concerning biogeochemical processes and also estimates of climate forcing and response. References [1] Swap R et al 1992 Saharan dust in the Amazon basin Tellus B 44 133-49 (doi:10.1034/j.1600-0889.1992.t01-1-00005.x) [2] Kaufman Y J, Koren I, Remer L A, Tanré D, Ginoux P and Fan S 2005 Dust transport and deposition observed from the Terra-MODIS space observations J. Geophys. Res. 110 D10S12 (doi:10.1029/2003JD004436) [3] Meskhidze N, Chameides W L and Nenes A 2005 Dust and pollution: a recipe for enhanced ocean fertizilation? J. Geophys. Res. 110 (D3) D03301 (doi:10.1029/2004JD005082) [4] Cakur R V et al 2006 Constraining the magnitude of the global dust cycle by minimizing the difference between a model and observations J. Geophys. Res. 111 D06207 (doi:10.1029/2005JD005791) [5] Ginoux P et al 2001 Sources and distribution of dust aerosol simulated with the GOCART model J. Geophys. Res. 106 20255-74 (doi:10.1029/2000JD000053) [6] Prospero J M, Ginoux P, Torres O, Nicholson S E and Gill T E 2002 Environmental characterization of global sources of atmospheric soil dust identified with the NIMBUS 7 total Ozone Mapping Spectrometer (TOMS) absorbing aerosol product Rev. Geophys. 40 (1) 1002 (doi:10.1029/2000RG000095) [7] Koren I, Kaufman Y J, Washington R, Todd M C, Rudich Y, Martins J V and Rosenfeld D 2006 The Bodélé depression: a single spot in the Sahara that provides most of the mineral dust to the Amazon forest Environ. Res Lett. 1 014005 (doi:10.1088/1748-9326/1/1/014005) Photo of Lorraine A Remer Lorraine A Remer received a BS degree in atmospheric science from the University of California, Davis, in 1980, an MS degree in oceanography from the Scripps Institution of Oceanography, University of California, San Diego, in 1983, and a PhD degree, also in atmospheric science from the University of California, Davis, in 1991. She became involved with the MODIS retrievals of atmospheric aerosols in 1991, first as a Research Scientist with Science Systems and Applications, Inc., and subsequently with the National Aeronautics and Space Administration, which she joined in 1998. She is an Associate Member of the MODIS Science Team and a Member of the Global Aerosol Climatology Project Science Team.

Comparison of the mixing state of long-range transported Asian and African mineral dust

NASA Astrophysics Data System (ADS)

Fitzgerald, Elizabeth; Ault, Andrew P.; Zauscher, Melanie D.; Mayol-Bracero, Olga L.; Prather, Kimberly A.

2015-08-01

Mineral dust from arid regions represents the second largest global source of aerosols to the atmosphere. Dust strongly impacts the radiative balance of the earth's atmosphere by directly scattering solar radiation and acting as nuclei for the formation of liquid droplets and ice nuclei within clouds. The climate effects of mineral dust aerosols are poorly understood, however, due to their complex chemical and physical properties, which continuously evolve during atmospheric transport. This work focuses on characterizing atmospheric mineral dust from the two largest global dust sources: the Sahara Desert in Africa and the Gobi and Taklamakan Deserts in Asia. Measurements of individual aerosol particle size and chemical mixing state were made at El Yunque National Forest, Puerto Rico, downwind of the Sahara Desert, and Gosan, South Korea, downwind of the Gobi and Taklamakan Deserts. In general, the chemical characterization of the individual dust particles detected at these two sites reflected the dominant mineralogy of the source regions; aluminosilicate-rich dust was more common at El Yunque (∼91% of El Yunque dust particles vs. ∼69% of Gosan dust particles) and calcium-rich dust was more common at Gosan (∼22% of Gosan dust particles vs. ∼2% of El Yunque dust particles). Furthermore, dust particles from Africa and Asia were subjected to different transport conditions and atmospheric processing; African dust showed evidence of cloud processing, while Asian dust was modified via heterogeneous chemistry and direct condensation of secondary species. A larger fraction of dust detected at El Yunque contained the cloud-processing marker oxalate ion compared to dust detected at Gosan (∼20% vs ∼9%). Additionally, nearly 100% of dust detected at Gosan contained nitrate, showing it was aged via heterogeneous reactions with nitric acid, compared to only ∼60% of African dust. Information on the distinct differences in the chemical composition of mineral dust particles, as well as the mechanisms and extent of atmospheric processing, is critical for assessing its impacts on the earth's radiative budget through scattering, absorption, and nucleating cloud droplets and ice crystals.

Removal of floating dust in glow discharge using plasma jet

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ticos, C. M.; Jepu, I.; Lungu, C. P.

2010-07-05

Dust can be an inconvenient source of impurities in plasma processing reactors and in many cases it can cause damage to the plasma-treated surfaces. A technique for dust expulsion out of the trapping region in plasma is presented here, based on the wind force exerted on dust particles by a pulsed plasma jet. Its applicability is demonstrated by removing floating dust in the sheath of parallel-plate capacitive radio-frequency plasma.

Cosmic dust

NASA Technical Reports Server (NTRS)

Brownlee, Donald E.; Sandford, Scott A.

1992-01-01

Dust is a ubiquitous component of our galaxy and the solar system. The collection and analysis of extraterrestrial dust particles is important to exobiology because it provides information about the sources of biogenically significant elements and compounds that accumulated in distant regions of the solar nebula and that were later accreted on the planets. The topics discussed include the following: general properties of interplanetary dust; the carbonaceous component of interplanetary dust particles; and the presence of an interstellar component.

High Proportions of Sub-micron Particulate Matter in Icelandic Dust Storms in 2015

NASA Astrophysics Data System (ADS)

Dagsson Waldhauserova, Pavla; Arnalds, Olafur; Olafsson, Haraldur; Magnusdottir, Agnes

2017-04-01

Iceland is extremely active dust region and desert areas of over 44,000 km2 acknowledge Iceland as the largest Arctic and European desert. Frequent dust events, up to 135 dust days annually, transport dust particles far distances towards the Arctic and Europe. Satellite MODIS pictures have revealed dust plumes exceeding 1,000 km. The annual dust deposition was calculated as 40.1 million tons yr-1. Two dust storms were measured in transverse horizontal profile about 90 km far from different dust sources in southwestern Iceland in the summer of 2015. Aerosol monitor DustTrak DRX 8533EP was used to measure PM mass concentrations corresponding to PM1, PM2.5, PM4, PM10 and the total PM15 at several places within the dust plume. Images from camera network operated by the Icelandic Road and Coastal Administration were used to estimate the visibility and spatial extent of measured dust events. A numerical simulation of surface winds was carried out with the numerical model HIRLAM with horizontal resolution of 5 km and used to calculate the total dust flux from the sources. The in situ measurements inside the dust plumes showed that aeolian dust can be very fine. The study highlights that suspended volcanic dust in Iceland causes air pollution with extremely high PM1 concentrations comparable to the polluted urban stations in Europe or Asia rather than reported dust event observations from around the world. The PM1/PM2.5 ratios are generally low during dust storms outside of Iceland, much lower than > 0.9 and PM1/PM10 ratios of 0.34-0.63 found in our study. It shows that Icelandic volcanic dust consists of higher proportion of submicron particles compared to crustal dust. The submicron particles are predicted to travel long distances. Moreover, such submicron particles pose considerable health risk because of high potential for entering the lungs. Icelandic volcanic glass has often fine pipe-vesicular structures known from asbestos and high content of heavy metals. Previous in situ measurements at the dust source in 2013 revealed extremely high number concentrations of submicron particles, specifically in the size range 0.3-0.337 μm. The PM2.5/PM10 ratios of mass concentrations seem to be lower at the dust sources that in some distance from the sources as measured in 2015. Common dust storms in Iceland are of several hundred thousand tons of magnitude from relatively well defined main dust sources. Numerical simulations were used calculate the total dust flux from the sources as 180,000 - 280,000 tons in this study. The mean PM1 (PM10) concentrations inside of the dust plumes varied from 97 to 241 µg m-3 (PM10 = 158 to 583 µg m-3). The extent of moderate dust events was calculated as 2.450 km2 to 4.220 km2 of the land area suggesting the regional scale of the events. Dust plumes reported here passed the most densely inhabited areas of Iceland, health risk warnings for the general public were, however, not issued. The data provided stresses the need for such warning system and is an important step towards its development.

Composition and sources of atmospheric dusts in snow at 3200 meters in the St. Elias Range, southeastern Alaska, USA

USGS Publications Warehouse

Hinkley, T.K.

1994-01-01

Dusts in snow from the accumulation zone in the St. Elias Range appear from their chemical compositions to have come from terranes of rocks of ferromagnesian composition. These dusts, with respect to their composition and to the moderate degree of variation that occurs through a depositional year, are similar those deposited in Greenland. The high portion of the St. Elias Range is isolated from dominance by any local dust source terranes, because of altitude and the extent of the surrounding glacierized and snow-covered region. In Greenland the altitude is typically lower, but local sources are even less likely to dominate the character of the dusts deposited into the ice record there. The similar compositions and moderate compositional variations of dusts from these two places bear on the question of whether the dusts that are transported over long distances by the atmosphere under modern and glacial-period conditions are uniform and representative of a broad regional or even hemispheric background dust. The dusts in the snow were measured by means of a suite of major, minor, and trace rock-forming metals chosen to give information about rock types, their constituent minerals, degree of degradation (weathering), and energies of atmospheric uptake from source. The variations in amounts of rock dust through the year in the St. Elias Range snowpack have no time-stratigraphic correspondence to the also large variations in concentrations of other species that are not constituents of rock-derived dusts, such the anions chloride, sulfate, and nitrate; the highs and lows of the two types of materials are apparently completely independent. The structure revealed by the moderately fine-scale sampling of the present study (??? 10 increments/y) serves as a background for the interpretation of analysis of ice core samples, in which annual layers may be too compressed to permit analysis of sub-annual samples. ?? 1994.

Composition and sources of atmospheric dusts in snow at 3200 meters in the St. Elias Range, southeastern Alaska, USA

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hinkley, T.K.

1994-08-01

Dusts in snow from the accumulation zone in the St. Elias Range appear from their chemical compositions to have come from terranes of rocks of ferromagnesian composition. These dusts, with respect to their composition and to the moderate degree of variation that occurs through a depositional year, are similar to those deposited in Greenland. The high portion of the St. Elias Range is isolated from dominance by any local dust source terranes, because of altitude and the extent of the surrounding glacierized and snow-covered region. In Greenland the altitude is typically lower, but local sources are even less likely tomore » dominate the character of the dusts deposited into the ice record there. The similar compositions and moderate compositional variations of dusts from these two places bear on the question of whether the dusts that are transported over long distances by the atmosphere under modern and glacial-period conditions are uniform and representative of a broad regional or even hemispheric background dust. The dusts in the snow were measured by means of a suite of major, minor, and track rock-forming metals chosen to give information about rock types, their constituent minerals, degree of degradation (weathering), and energies of atmospheric uptake from source. The variations in amounts of rock dust through the year in the St. Elias Range snowpack have no time-stratigraphic correspondence to the also-large variations in concentrations of other species that are not constituents of rock-derived dusts, such the anions chloride, sulfate, and nitrate; the highs and lows of the two types of materials are apparently completely independent. The structure revealed by the moderately fine-scale sampling of the present study ([approximately]10 increments/y) serves as a background for the interpretation of analysis of ice core samples, in which annual layers may be too compressed to permit analysis of sub-annual samples.« less

The infrared spectrum of M8 E - Evidence for circumstellar CO

NASA Technical Reports Server (NTRS)

Larson, H. P.; Fink, U.; Hofmann, R.

1986-01-01

High-resolution spectroscopic observations of the compact infrared source M8 E are reported in the region from 3 to 5 microns. Very prominent CO absorption lines are observed in the v = 1-0 band at 4.7 microns. The velocity width and rotational temperature suggest that this CO absorption occurs in a highly excited region. The high background continuum flux level and the prominent appearance of the CO features suggest that the CO line-forming region must be in front of the dust emission region. A blister model for M8 E, which places most of the dust continuum emission behind the source, satisfies this requirement. According to this picture, the observed circumstellar CO spectrum shows a high rotational temperature and a large velocity dispersion because of the combined effects of the strong stellar wind and possible shock heating near the dust zone as the wind encounters the ambient molecular cloud.

African Dust Aerosols as Atmospheric Ice Nuclei

NASA Technical Reports Server (NTRS)

DeMott, Paul J.; Brooks, Sarah D.; Prenni, Anthony J.; Kreidenweis, Sonia M.; Sassen, Kenneth; Poellot, Michael; Rogers, David C.; Baumgardner, Darrel

2003-01-01

Measurements of the ice nucleating ability of aerosol particles in air masses over Florida having sources from North Africa support the potential importance of dust aerosols for indirectly affecting cloud properties and climate. The concentrations of ice nuclei within dust layers at particle sizes below 1 pn exceeded 1/cu cm; the highest ever reported with our device at temperatures warmer than homogeneous freezing conditions. These measurements add to previous direct and indirect evidence of the ice nucleation efficiency of desert dust aerosols, but also confirm their contribution to ice nuclei populations at great distances from source regions.

Characteristics and transport of organochlorine pesticides in urban environment: air, dust, rain, canopy throughfall, and runoff.

PubMed

Zhang, Wei; Ye, Youbin; Hu, Dan; Ou, Langbo; Wang, Xuejun

2010-11-01

Characteristics and transport of organochlorine pesticides (OCPs) in urban multiple environments, including air, dust, rain, canopy throughfall, and runoff water, are explored in this study. Hexachlorocyclohexanes (HCHs) dominated in both air and rain water, and dichlorodiphenyltrichloroethane (DDT) related substances showed a higher affinity to dust. Relatively high concentrations of DDT and dichlorodiphenyldichloroethylene (DDE) in air, rain and dust imply that technical DDT in the environment has been degrading, and there may be unknown local or regional emission sources that contain DDTs in the study area. Source identification showed that DDTs in Beijing urban environments with a fresh signature may originate from the atmospheric transport from remote areas. The ratio of α-/γ-HCH in dust, rain, canopy throughfall and runoff were close to 1, indicating the possible use of lindane. OCPs in runoff were transported from various sources including rain, dust, and canopy throughfall. In runoff, DDTs and hexachlorobenzene (HCB) were mainly transported from dust, and HCHs were mainly from rain and canopy throughfall.

Mineral dust emission from the Bodélé Depression, northern Chad, during BoDEx 2005

NASA Astrophysics Data System (ADS)

Todd, Martin C.; Washington, Richard; Martins, José Vanderlei; Dubovik, Oleg; Lizcano, Gil; M'bainayel, Samuel; Engelstaedter, Sebastian

2007-03-01

Mineral dust in the atmosphere is an important component of the climate system but is poorly quantified. The Bodélé Depression of northern Chad stands out as the world's greatest source region of mineral dust into the atmosphere. Frequent dust plumes are a distinguishing feature of the region's climate. There is a need for more detailed information on processes of dust emission/transport and dust optical properties to inform model simulations of this source. During the Bodélé Dust Experiment (BoDEx) in 2005, instrumentation was deployed to measure dust properties and boundary layer meteorology. Observations indicate that dust emission events are triggered when near-surface wind speeds exceed 10 ms-1, associated with synoptic-scale variability in the large-scale atmospheric circulation. Dust emission pulses in phase with the diurnal cycle of near-surface winds. Analysis of dust samples shows that the dust consists predominantly of fragments of diatomite sediment. The particle size distribution of this diatomite dust estimated from sun photometer data, using a modified Aeronet retrieval algorithm, indicates a dominant coarse mode (radius centered on 1-2 μm) similar to other Saharan dust observations. Single-scattering albedo values are high, broadly in line with other Saharan dust even though the diatomite composition of dust from the Bodélé is likely to be unusual. The radiative impact of high dust loadings results in a reduction in surface daytime maximum temperature of around 7°C in the Bodélé region. Using optical and physical properties of dust obtained in the field, we estimate the total dust flux emitted from the Bodélé to be 1.18 ± 0.45 Tg per day during a substantial dust event. We speculate that the Bodélé Depression (˜10,800 km2) may be responsible for between 6-18% of global dust emissions, although the uncertainty in both the Bodélé and global estimates remains high.

Impact of Asian Dust on Climate and Air Quality

NASA Technical Reports Server (NTRS)

Chin, Mian; Tan, Qian; Diehl, Thomas; Yu, Hongbin

2010-01-01

Dust generated from Asian permanent desert and desertification areas can be efficiently transported around the globe, making significant radiative impact through their absorbing and scattering solar radiation and through their deposition on snow and ice to modify the surface albedo. Asian dust is also a major concern of surface air quality not only in the source and immediate downwind regions but also areas thousands of miles away across the Pacific. We present here a global model, GOCART, analysis of data from satellite remote sensing instrument (MODIS, MISR, CALIPSO, OMI) and other observations on Asian dust sources, transport, and deposition, and use the model to assess the Asian dust impact on global climate and air quality.

The dusty ballerina skirt of Jupiter

NASA Astrophysics Data System (ADS)

Horanyi, M.; Morfill, G.; Gruen, E.

1993-12-01

We suggest a model to explain the unexpected recurrent dust events that were observed during the Jupiter encounter by the dust detector on board the Ulysses spacecraft. This model is based dust-magnetosphere interactions. Dust particles inside the Jovian magnetosphere collect electrostatic charges and their interaction with the magnetic and electric fields can lead to energization and subsequent ejection. We discuss the dusty regions (ring/halo, `gossamer' ring) and also Io as potential sources for the Ulysses events. This model favors Io as a source. The mass and velocity range of the escaping particles are compatible with the observations, and we also suggest internal periodicities to explain the recurrent nature of the Ulysses dust events.

Mineral dust: observations of emission events and modeling of transport to the upper troposphere

NASA Astrophysics Data System (ADS)

Peter, T.; Wiacek, A.; Taddeo, M.

2009-04-01

The present study explores differences between mineral dust emission events in West African and Asian (Taklimakan) deserts, focusing on the availability of bare mineral dust ice nuclei for interactions with cirrus clouds without previous processing or washout by liquid water clouds. One-week trajectory calculations with high-resolution ECMWF fields are used to track transported (Lagrangian) relative humidities with respect to liquid water and ice, allowing to estimate the formation of liquid, mixed-phase and ice clouds. Transport trajectories can reasonably be assumed to carry dust with them throughout the year, except for the months of December-February, which are quiescent with respect to dust emission in both regions. Practically none of the simulated air parcels reach regions where homogeneous nucleation can take place (T < -35°C) along trajectories that have not experienced water saturation first, i.e. it is very unlikely that mineral dust particles could be a serious competitor for homogeneous nucleation during the formation of high, cold cirrus clouds. For the temperature region between -35°C < T < 0°C, i.e. in air parcels exhibiting necessary conditions for warmer ice clouds at lower altitudes, a small but significant number of air parcels are found to follow trajectories where RHw < 100% and RHi > 100% are simultaneously maintained. However, the potential for such low ice clouds originating from the Taklimakan desert is greater than that of the Sahara by a factor of 4-6. The implication is that although the Sahara is by far the biggest source of dust in the world, the much smaller Taklimakan desert in China's Tarim Basin may be of greater importance as a source of ice nuclei affecting cirrus cloud formation. This is likely the result of several meteorological factors, including the complex regional topography combined with the higher altitude of Taklimakan dust emissions and, on the synoptic scale, the higher altitude of potential temperature levels in the free troposphere at mid-latitudes than in the tropics. Finally, the very active Bodélé source region in Africa and the Gobi Desert in Asia will also be addressed.

Complex molecules in Sagittarius B2(N): The importance of grain chemistry

NASA Technical Reports Server (NTRS)

Miao, Yanti; Mehringer, David M.; Kuan, Yi-Jheng; Snyder, Lewis E.

1995-01-01

The complex molecules vinyl cyanide (CH2CHCN), methyl formate (HCOOCH3), and ethyl cyanide (CH3CH2CN) were observed in the Sgr B2 star-forming region with the BIMA millimeter wavelength array. A region with diameter less than 0.1 pc toward the Sgr B2(N) molecular core is found to be the major source of these molecules. Also, this source is coincident with continuum emission from dust and a center of H2O maser activity. Ultracompact (UC) H 11 regions are located within 0.1 pc. Strikingly, none of these molecules is detected toward Sgr B2(M), a core located 1 minute south of Sgr B2(N). The existence of complex molecules, a large mass of dust, high-velocity H2O masers, and UC H 11 regions strongly suggests that the Sgr B2(N) region has just begun to form stars, while the absence of strong dust emission and large molecules suggests Sgr B2(M) is more evolved. The detection of large molecules coincident with continuum emission from dust supports the idea found in current chemical models that grain chemistry is of crucial importance for the formation of these molecules.

Assessment of State-of-the-Art Dust Emission Scheme in GEOS

NASA Technical Reports Server (NTRS)

Darmenov, Anton; Liu, Xiaohong; Prigent, Catherine

2017-01-01

The GEOS modeling system has been extended with state of the art parameterization of dust emissions based on the vertical flux formulation described in Kok et al 2014. The new dust scheme was coupled with the GOCART and MAM aerosol models. In the present study we compare dust emissions, aerosol optical depth (AOD) and radiative fluxes from GEOS experiments with the standard and new dust emissions. AOD from the model experiments are also compared with AERONET and satellite based data. Based on this comparative analysis we concluded that the new parameterization improves the GEOS capability to model dust aerosols originating from African sources, however it lead to overestimation of dust emissions from Asian and Arabian sources. Further regional tuning of key parameters controlling the threshold friction velocity may be required in order to achieve more definitive and uniform improvement in the dust modeling skill.

Stable Isotopes of Sr and Pb as Tracers of Sources of Airborne Particulate Matter in Kyrgyzstan

EPA Science Inventory

ConclusionsElemental concentrations were higher at the LIDAR site compared to the Bishkek site. Also, concentrations were higher during dust than non-dust events at both sites.The Sr isotopic ratios suggest dust from another region, such as from Western China, Africa, or Middle E...

A radiogenic isotope tracer study of transatlantic dust transport from Africa to the Caribbean

NASA Astrophysics Data System (ADS)

Kumar, A.; Abouchami, W.; Galer, S. J. G.; Garrison, V. H.; Williams, E.; Andreae, M. O.

2014-01-01

Many studies have suggested that long-range transport of African desert dusts across the Atlantic Ocean occurs, delivering key nutrients and contributing to fertilization of the Amazon rainforest. Here we utilize radiogenic isotope tracers - Sr, Nd and Pb - to derive the provenance, local or remote, and pathways of dust transport from Africa to the Caribbean. Atmospheric total suspended particulate (TSP) matter was collected in 2008 on quartz fibre filters, from both sides of the Atlantic Ocean at three different locations: in Mali (12.6°N, 8.0°W; 555 m a.s.l.), Tobago (11.3°N, 60.5°W; 329 m a.s.l.) and the U.S. Virgin Islands (17.7°N, 64.6°W; 27 m a.s.l.). Both the labile phase, representative of the anthropogenic signal, and the refractory detrital silicate fraction were analysed. Dust deposits and soils from around the sampling sites were measured as well to assess the potential contribution from local sources to the mineral dust collected. The contribution from anthropogenic sources of Pb was predominant in the labile, leachate phase. The overall similarity in Pb isotope signatures found in the leachates is attributed to a common African source of anthropogenic Pb, with minor inputs from other sources, such as from Central and South America. The Pb, Sr and Nd isotopic compositions in the silicate fraction were found to be systematically more radiogenic than those in the corresponding labile phases. In contrast, Nd and Sr isotopic compositions from Mali, Tobago, and the Virgin Islands are virtually identical in both leachates and residues. Comparison with existing literature data on Saharan and Sahelian sources constrains the origin of summer dust transported to the Caribbean to mainly originate from the Sahel region, with some contribution from northern Saharan sources. The source regions derived from the isotope data are consistent with 7-day back-trajectory analyses, demonstrating the usefulness of radiogenic isotopes in tracing dust provenance and atmospheric transport.

Top-down estimate of dust emissions through integration of MODIS and MISR aerosol retrievals with the GEOS-Chem adjoint model

NASA Astrophysics Data System (ADS)

Wang, Jun; Xu, Xiaoguang; Henze, Daven K.; Zeng, Jing; Ji, Qiang; Tsay, Si-Chee; Huang, Jianping

2012-04-01

Predicting the influences of dust on atmospheric composition, climate, and human health requires accurate knowledge of dust emissions, but large uncertainties persist in quantifying mineral sources. This study presents a new method for combined use of satellite-measured radiances and inverse modeling to spatially constrain the amount and location of dust emissions. The technique is illustrated with a case study in May 2008; the dust emissions in Taklimakan and Gobi deserts are spatially optimized using the GEOS-Chem chemical transport model and its adjoint constrained by aerosol optical depth (AOD) that are derived over the downwind dark-surface region in China from MODIS (Moderate Resolution Imaging Spectroradiometer) reflectance with the aerosol single scattering properties consistent with GEOS-chem. The adjoint inverse modeling yields an overall 51% decrease in prior dust emissions estimated by GEOS-Chem over the Taklimakan-Gobi area, with more significant reductions south of the Gobi Desert. The model simulation with optimized dust emissions shows much better agreement with independent observations from MISR (Multi-angle Imaging SpectroRadiometer) AOD and MODIS Deep Blue AOD over the dust source region and surface PM10 concentrations. The technique of this study can be applied to global multi-sensor remote sensing data for constraining dust emissions at various temporal and spatial scales, and hence improving the quantification of dust effects on climate, air quality, and human health.

Top-down Estimate of Dust Emissions Through Integration of MODIS and MISR Aerosol Retrievals With the Geos-chem Adjoint Model

NASA Technical Reports Server (NTRS)

Wang, Jun; Xu, Xiaoguang; Henze, Daven K.; Zeng, Jing; Ji, Qiang; Tsay, Si-Chee; Huang, Jianping

2012-01-01

Predicting the influences of dust on atmospheric composition, climate, and human health requires accurate knowledge of dust emissions, but large uncertainties persist in quantifying mineral sources. This study presents a new method for combined use of satellite-measured radiances and inverse modeling to spatially constrain the amount and location of dust emissions. The technique is illustrated with a case study in May 2008; the dust emissions in Taklimakan and Gobi deserts are spatially optimized using the GEOSChem chemical transport model and its adjoint constrained by aerosol optical depth (AOD) that are derived over the downwind dark-surface region in China from MODIS (Moderate Resolution Imaging Spectroradiometer) reflectance with the aerosol single scattering properties consistent with GEOS-chem. The adjoint inverse modeling yields an overall 51% decrease in prior dust emissions estimated by GEOS-Chem over the Taklimakan-Gobi area, with more significant reductions south of the Gobi Desert. The model simulation with optimized dust emissions shows much better agreement with independent observations from MISR (Multi-angle Imaging SpectroRadiometer) AOD and MODIS Deep Blue AOD over the dust source region and surface PM10 concentrations. The technique of this study can be applied to global multi-sensor remote sensing data for constraining dust emissions at various temporal and spatial scales, and hence improving the quantification of dust effects on climate, air quality, and human health.

Long-term aerosol measurements in Gran Canaria, Canary Islands: Particle concentration, sources and elemental composition

NASA Astrophysics Data System (ADS)

Gelado-Caballero, MaríA. D.; López-GarcíA, Patricia; Prieto, Sandra; Patey, Matthew D.; Collado, Cayetano; HéRnáNdez-Brito, José J.

2012-02-01

There are very few sets of long-term measurements of aerosol concentrations over the North Atlantic Ocean, yet such data is invaluable in quantifying atmospheric dust inputs to this ocean region. We present an 8-year record of total suspended particles (TSP) collected at three stations on Gran Canaria Island, Spain (Taliarte at sea level, Tafira 269 m above sea level (a.s.l.) and Pico de la Gorra 1930 m a.s.l.). Using wet and dry deposition measurements, the mean dust flux was calculated at 42.3 mg m-2 d-1. Air mass back trajectories (HYSPLIT, NOAA) suggested that the Sahara desert is the major source of African dust (dominant during 32-50% of days), while the Sahel desert was the major source only 2-10% of the time (maximum in summer). Elemental composition ratios of African samples indicate that, despite the homogeneity of the dust in collected samples, some signatures of the bedrocks can still be detected. Differences were found for the Sahel, Central Sahara and North of Sahara regions in Ti/Al, Mg/Al and Ca/Al ratios, respectively. Elements often associated with pollution (Pb, Cd, Ni, Zn) appeared to share a common origin, while Cu may have a predominantly local source, as suggested by a decrease in the enrichment factor (EF) of Cu during dust events. The inter-annual variability of dust concentrations is investigated in this work. During winter, African dust concentration measurements at the Pico de la Gorra station were found to correlate with the North Atlantic Oscillation (NAO) index.

Influence of regional biomass burning on the highly elevated organic carbon concentrations observed at Gosan, South Korea during a strong Asian dust period.

PubMed

Nguyen, Duc Luong; Kim, Jin Young; Ghim, Young Sung; Shim, Shang-Gyoo

2015-03-01

PM2.5 carbonaceous particles were measured at Gosan, South Korea during 29 March-11 April 2002 which includes a pollution period (30 March-01 April) when the highest concentrations of major anthropogenic species (nss-SO4 (2-), NO3 (-), and NH4 (+)) were observed and a strong Asian dust (AD) period (08-10 April) when the highest concentrations of mainly dust-originated trace elements (Al, Ca, Mg, and Fe) were seen. The concentrations of elemental carbon (EC) measured in the pollution period were higher than those measured in the strong AD period, whereas an inverse variation in the concentrations of organic carbon (OC) was observed. Based on the OC/EC ratios, the possible source that mainly contributed to the highly elevated OC concentrations measured in the strong AD period was biomass burning. The influence of the long-range transport of smoke plumes emitted from regional biomass burning sources was evaluated by using MODIS (Moderate Resolution Imaging Spectroradiometer) satellite data for fire locations and the potential source contribution function analysis. The most potential source regions of biomass burning were the Primorsky and Amur regions in Far Eastern Russia and southeastern and southwestern Siberia, Russia. Further discussion on the source characteristics suggested that the high OC concentrations measured in the strong AD period were significantly affected by the smoldering phase of biomass burning. In addition to biomass burning, secondary OC (SOC) formed during atmospheric long-range transport should be also considered as an important source of OC concentration measured at Gosan. Although this study dealt with the episodic case of the concurrent increase of dust and biomass burning particles, understanding the characteristics of heterogeneous mixing aerosol is essential in assessing the radiative forcing of aerosol.

Coupled European and Greenland last glacial dust activity driven by North Atlantic climate

PubMed Central

Stevens, Thomas; Molnár, Mihály; Demény, Attila; Lambert, Fabrice; Varga, György; Páll-Gergely, Barna; Buylaert, Jan-Pieter; Kovács, János

2017-01-01

Centennial-scale mineral dust peaks in last glacial Greenland ice cores match the timing of lowest Greenland temperatures, yet little is known of equivalent changes in dust-emitting regions, limiting our understanding of dust−climate interaction. Here, we present the most detailed and precise age model for European loess dust deposits to date, based on 125 accelerator mass spectrometry 14C ages from Dunaszekcső, Hungary. The record shows that variations in glacial dust deposition variability on centennial–millennial timescales in east central Europe and Greenland were synchronous within uncertainty. We suggest that precipitation and atmospheric circulation changes were likely the major influences on European glacial dust activity and propose that European dust emissions were modulated by dominant phases of the North Atlantic Oscillation, which had a major influence on vegetation and local climate of European dust source regions. PMID:29180406

Compositions of modern dust and surface sediments in the Desert Southwest, United States

USGS Publications Warehouse

Reheis, M.C.; Budahn, J.R.; Lamothe, P.J.; Reynolds, R.L.

2009-01-01

Modern dusts across southwestern United States deserts are compositionally similar to dust-rich Av soil horizons (depths of 0-0.5 cm and 1-4 cm at 35 sites) for common crustal elements but distinctly different for some trace elements. Chemical compositions and magnetic properties of the soil samples are similar among sites relative to dust sources, geographic areas, and lithologic substrates. Exceptions are Li, U, and W, enriched in Owens Valley, California, and Mg and Sr, enriched in soils formed on calcareous fan gravel in southeast Nevada. The Av horizons are dominated by dust and reflect limited mixing with substrate sediments. Modern dust samples are also similar across the region, except that Owens Valley dusts are higher in Mg, Ba, and Li and dusts both there and at sites to the north on volcanic substrates are higher in Sb and W. Thus, dust and Av horizons consist of contributions from many different sources that are well mixed before deposition. Modern dusts contain significantly greater amounts of As, Cd, Cr, Cu, Ni, Pb, and Sb than do Av horizons, which record dust additions over hundreds to thousands of years. These results suggest that modern dust compositions are influenced by anthropogenic sources and emissions from Owens (dry) Lake after its artificial desiccation in 1926. Both modern dusts and Av horizons are enriched in As, Ba, Cu, Li, Sb, Th, U, and W relative to average crustal composition, which we interpret to indicate that the geologic sources of dust in the southwestern United States are geochemically distinctive.

The Impact of Desert Dust Aerosol Radiative Forcing on Global and West African Precipitation

NASA Astrophysics Data System (ADS)

Jordan, A.; Zaitchik, B. F.; Gnanadesikan, A.; Dezfuli, A. K.

2015-12-01

Desert dust aerosols exert a radiative forcing on the atmosphere, influencing atmospheric temperature structure and modifying radiative fluxes at the top of the atmosphere (TOA) and surface. As dust aerosols perturb radiative fluxes, the atmosphere responds by altering both energy and moisture dynamics, with potentially significant impacts on regional and global precipitation. Global Climate Model (GCM) experiments designed to characterize these processes have yielded a wide range of results, owing to both the complex nature of the system and diverse differences across models. Most model results show a general decrease in global precipitation, but regional results vary. Here, we compare simulations from GFDL's CM2Mc GCM with multiple other model experiments from the literature in order to investigate mechanisms of radiative impact and reasons for GCM differences on a global and regional scale. We focus on West Africa, a region of high interannual rainfall variability that is a source of dust and that neighbors major Sahara Desert dust sources. As such, changes in West African climate due to radiative forcing of desert dust aerosol have serious implications for desertification feedbacks. Our CM2Mc results show net cooling of the planet at TOA and surface, net warming of the atmosphere, and significant increases in precipitation over West Africa during the summer rainy season. These results differ from some previous GCM studies, prompting comparative analysis of desert dust parameters across models. This presentation will offer quantitative analysis of differences in dust aerosol parameters, aerosol optical properties, and overall particle burden across GCMs, and will characterize the contribution of model differences to the uncertainty of forcing and climate response affecting West Africa.

Influence of Complex Terrain on Wind Fields in the Mojave Desert, Southwestern US

NASA Astrophysics Data System (ADS)

Clow, G. D.; Reynolds, R. L.; Urban, F. E.; Bogle, R.; Vogel, J. M.

2009-12-01

The complex terrain of southern California has important effects on the winds in this dust-producing region. We use the Weather Research and Forecasting Model (WRF) to investigate the influences of rugged topography on the wind field in the Mojave Desert at a variety of scales. For this study, the WRF model was used in a retrospective mode over the time period 2000-to-present, with horizontal resolutions as fine as 1-km in specific areas of interest (i.e., known dust-source areas). At a regional scale, the juxtaposition of California's Central Valley with the Sierra Nevada Mountain Range often generates a band of strong winds extending eastward from the southern end of the Sierra Nevada and Tehachapi Mountains across the Mojave Desert and into Arizona. At finer scales, WRF-derived winds within this band reveal terrain deflection, focusing, channeling, and rapid direction change over short distances. These effects are important for assessing the capacity of wind to produce dust at potential dust-source areas during specific events, and for determining dust-transport pathways. Comparison of the WRF results during strong wind events with data from meteorological stations having dust emission instruments (saltation sensors and/or wind-triggered time-lapse cameras) help elucidate landscape conditions that influence dust emission and patterns of dust transport.

Ice Nucleating Particle Properties in the Saharan Air Layer Close to the Dust Source

NASA Astrophysics Data System (ADS)

Boose, Y.; Garcia, I. M.; Rodríguez, S.; Linke, C.; Schnaiter, M.; Nickovic, S.; Lohmann, U.; Kanji, Z. A.; Sierau, B.

2015-12-01

In August 2013 and 2014 measurements of ice nucleating particle (INP) concentrations, aerosol particle size distributions, chemistry and fluorescence were conducted at the Izaña Atmospheric Observatory located at 2373 m asl on Tenerife, west off the African shore. During summer, the observatory is frequently within the Saharan Air Layer and thus often exposed to dust. Absolute INP concentrations and activated fractions at T=-40 to -15°C and RHi=100-150 % were measured. In this study, we discuss the in-situ measured INP properties with respect to changes in the chemical composition, the biological content, the source regions as well as transport pathways and thus aging processes of the dust aerosol. For the first time, ice crystal residues were also analyzed with regard to biological content by means of their autofluorescence signal close to a major dust source region. Airborne dust samples were collected with a cyclone for additional offline analysis in the laboratory under similar conditions as in the field. Both, in-situ and offline dust samples were chemically characterized using single-particle mass spectrometry. The DREAM8 dust model extended with dust mineral fractions was run to simulate meteorological and dust aerosol conditions for ice nucleation. Results show that the background aerosol at Izaña was dominated by carbonaceous particles, which were hardly ice-active under the investigated conditions. When Saharan dust was present, INP concentrations increased by up to two orders of magnitude even at water subsaturated conditions at T≤-25°C. Differences in the ice-activated fraction were found between different dust periods which seem to be linked to variations in the aerosol chemical composition (dust mixed with changing fractions of sea salt and differences in the dust aerosol itself). Furthermore, two biomass burning events in 2014 were identified which led to very low INP concentrations under the investigated temperature and relative humidity conditions.

Use of MODIS Satellite Images and an Atmospheric Dust Transport Model to Evaluate Juniperus spp. Pollen Phenology and Dispersal

NASA Technical Reports Server (NTRS)

Luvall, J. C.; Sprigg, W. A.; Levetin, E.; Huete, A.; Nickovic, S.; Pejanovic, G. A.; Vukovic, A.; VandeWater, P. K.; Myers, O. B.; Budge, A. M.;

Characterization of Dust Properties at the Source Region During ACE-Asia

NASA Technical Reports Server (NTRS)

Tsay, Si-Chee; Lau, William (Technical Monitor)

2001-01-01

ACE (Aerosol Characterization Experiment)-Asia is designed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally-occurring aerosols, which often exist in high concentrations over eastern Asia and along the rim of the western Pacific. The phase-I of ACE-Asia was conducted from March-May 2001 in the vicinity of the Gobi desert, east coast of China, Yellow Sea, Korea, and Japan, along the pathway of Kosa (severe events that blanket East Asia with yellow desert dust, peaked in the Spring season). Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian dust is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia we have measured continuously aerosol optical/radiative properties, column precipitable water amount, and surface reflectivity over homogeneous areas from surface. The inclusion of flux measurements permits the determination of dust aerosol radiative flux in addition to measurements of loading and optical thickness. At the time of the Terra/MODIS overpass, these ground-based observations can provide valuable data to compare with MODIS retrievals over land. Preliminary results will be presented and discussed their implications in regional climatic effects.

Dust Emissions, Transport, and Deposition Simulated with the NASA Finite-Volume General Circulation Model

NASA Technical Reports Server (NTRS)

Colarco, Peter; daSilva, Arlindo; Ginoux, Paul; Chin, Mian; Lin, S.-J.

2003-01-01

Mineral dust aerosols have radiative impacts on Earth's atmosphere, have been implicated in local and regional air quality issues, and have been identified as vectors for transporting disease pathogens and bringing mineral nutrients to terrestrial and oceanic ecosystems. We present for the first time dust simulations using online transport and meteorological analysis in the NASA Finite-Volume General Circulation Model (FVGCM). Our dust formulation follows the formulation in the offline Georgia Institute of Technology-Goddard Global Ozone Chemistry Aerosol Radiation and Transport Model (GOCART) using a topographical source for dust emissions. We compare results of the FVGCM simulations with GOCART, as well as with in situ and remotely sensed observations. Additionally, we estimate budgets of dust emission and transport into various regions.

Assessing sources of airborne mineral dust and other aerosols, in Iraq

NASA Astrophysics Data System (ADS)

Engelbrecht, Johann P.; Jayanty, R. K. M.

2013-06-01

Most airborne particulate matter in Iraq comes from mineral dust sources. This paper describes the statistics and modeling of chemical results, specifically those from Teflon® filter samples collected at Tikrit, Balad, Taji, Baghdad, Tallil and Al Asad, in Iraq, in 2006/2007. Methodologies applied to the analytical results include calculation of correlation coefficients, Principal Components Analysis (PCA), and Positive Matrix Factorization (PMF) modeling. PCA provided a measure of the covariance within the data set, thereby identifying likely point sources and events. These include airborne mineral dusts of silicate and carbonate minerals, gypsum and salts, as well as anthropogenic sources of metallic fumes, possibly from battery smelting operations, and emissions of leaded gasoline vehicles. Five individual PMF factors (source categories) were modeled, four of which being assigned to components of geological dust, and the fifth to gasoline vehicle emissions together with battery smelting operations. The four modeled geological components, dust-siliceous, dust-calcic, dust-gypsum, and evaporate occur in variable ratios for each site and size fraction (TSP, PM10, and PM2.5), and also vary by season. In general, Tikrit and Taji have the largest and Al Asad the smallest percentages of siliceous dust. In contrast, Al Asad has the largest proportion of gypsum, in part representing the gypsiferous soils in that region. Baghdad has the highest proportions of evaporite in both size fractions, ascribed to the highly salinized agricultural soils, following millennia of irrigation along the Tigris River valley. Although dust storms along the Tigris and Euphrates River valleys originate from distal sources, the mineralogy bears signatures of local soils and air pollutants.

Diagnostic evaluation of the Community Earth System Model in simulating mineral dust emission with insight into large-scale dust storm mobilization in the Middle East and North Africa (MENA)

NASA Astrophysics Data System (ADS)

Parajuli, Sagar Prasad; Yang, Zong-Liang; Lawrence, David M.

2016-06-01

Large amounts of mineral dust are injected into the atmosphere during dust storms, which are common in the Middle East and North Africa (MENA) where most of the global dust hotspots are located. In this work, we present simulations of dust emission using the Community Earth System Model Version 1.2.2 (CESM 1.2.2) and evaluate how well it captures the spatio-temporal characteristics of dust emission in the MENA region with a focus on large-scale dust storm mobilization. We explicitly focus our analysis on the model's two major input parameters that affect the vertical mass flux of dust-surface winds and the soil erodibility factor. We analyze dust emissions in simulations with both prognostic CESM winds and with CESM winds that are nudged towards ERA-Interim reanalysis values. Simulations with three existing erodibility maps and a new observation-based erodibility map are also conducted. We compare the simulated results with MODIS satellite data, MACC reanalysis data, AERONET station data, and CALIPSO 3-d aerosol profile data. The dust emission simulated by CESM, when driven by nudged reanalysis winds, compares reasonably well with observations on daily to monthly time scales despite CESM being a global General Circulation Model. However, considerable bias exists around known high dust source locations in northwest/northeast Africa and over the Arabian Peninsula where recurring large-scale dust storms are common. The new observation-based erodibility map, which can represent anthropogenic dust sources that are not directly represented by existing erodibility maps, shows improved performance in terms of the simulated dust optical depth (DOD) and aerosol optical depth (AOD) compared to existing erodibility maps although the performance of different erodibility maps varies by region.

Stoichiometry of water-soluble ions in PM2.5: Application in source apportionment for a typical industrial city in semi-arid region, Northwest China

NASA Astrophysics Data System (ADS)

Zhou, Haijun; Lü, Changwei; He, Jiang; Gao, Manshu; Zhao, Boyi; Ren, Limin; Zhang, Lijun; Fan, Qingyun; Liu, Tao; He, Zhongxiang; Dudagula; Zhou, Bin; Liu, Hualin; Zhang, Yu

2018-05-01

Water-soluble ions (WSIs) are major components of PM2.5 and it is valuable for understanding physical and chemical characteristics, sources, behaviors and formation mechanism of WSIs. Baotou is a traditionally industrial city in semi-arid region and frequently subjected to dust storms from March to May. In recent years, air pollution has been listed as one of the most important environmental problems in Baotou. To investigate the seasonal variations and sources of WSIs in PM2.5, the WSIs including SO42-, NO3-, Cl-, F-, NH4+, K+, Na+, Ca2+ and Mg2+ were monitored at six urban sites in Baotou. The results showed that high concentrations of Ca2+ and Na+ were found responding to dust storm events, while high concentrations of SO42-, NO3-, NH4+, K+ and Cl- were observed during haze days. The correlations analysis indicated that excess sulfuric and nitric acid was likely neutralized by carbonate minerals such as calcite, aragonite and dolomite in normal days and cations were fully neutralized during all the sampling periods, while cations were excessive in dust storm days. The concentrations of [NH4+ + SO42- + NO3-], [Na+ + Ca2+ + Mg2+] and [Cl- + K+ + F-] indicated the northwest and southeast region of Baotou presented comparatively high contributions of secondary aerosol and crustal dust, respectively, which were mainly related to the industrial distribution and urbanization process. The cluster analysis, ternary diagram and principal component analysis have a good agreement in source apportionment, where crustal dust sources, secondary aerosol source and the mixture of coal combustion, biomass burning and industrial pollution sources were the main sources of WSIs in PM2.5. The seasonal pattern of sulfur oxidation ratio (SOR) was September > April > November > January, while the nitrogen oxidation ratio (NOR) April > January > November > September in Baotou. This work evaluated the seasonal variation, distribution and source of WSIs on the basis of its stoichiometry in PM2.5, which help to explore the potential sources of these inorganic aerosols and provide scientific suggestion for air quality improvement in Baotou.

Constant Chinese Loess Plateau dust source since the Late Miocene

NASA Astrophysics Data System (ADS)

Bird, Anna; Millar, Ian; Stevens, Thomas; Rodenburg, Tanja; Rittner, Martin; Vermeesch, Pieter; Lu, Huayu

2017-04-01

The dramatic deepening of northern hemisphere glaciation at the Pliocene-Pleistocene boundary is accompanied by major changes in global climate. The role of the global atmospheric dust cycle in this event is not clear; in particular, whether, changes in the dust cycle influenced climates change, or resulted from it. Miocene and Quaternary wind-blown Chinese loess records past dust-cycle history, influences of aridification and monsoon circulation. Previous work on the vast Chinese Loess Plateau is in conflict over whether changes in dust source occur at the Pliocene-Pleistocene boundary (2.59 Ma), or at 1.2 Ma, despite these intervals marking major shifts in monsoon dynamics (Sun 2005; Nie et al. 2014a). Here we present Sr, Nd and Hf isotopic data from multiple sites and show that the dust source remains the same across these boundaries. The use of isotope tracers from multiple sites allows us to demonstrate that shifts in sediment geochemistry can be explained by grain-size and weathering changes. Nd and Hf isotopes show that the dust was dominantly sourced from the Tibetan Plateau, with some input from bedrock underlying the Badain Jaran/Tengger deserts. This shows that a major established and constant dust source on the northern Tibetan Plateau has been active and unchanged since the late Miocene, despite dramatically changing climate conditions. Changes in loess accumulation are therefore a function of climate change in the Tibetan Plateau source regions rather than due to expanding source areas controlled by aridification over a widening area over the Pliocene and Quaternary.

Reconstruction of South Pacific Dust Accumulation during the Early Paleogene Greenhouse

NASA Astrophysics Data System (ADS)

Amaya, D.; Thomas, D. J.; Marcantonio, F.; Korty, R.; Huber, M.; Winckler, G.; Alvarez Zarikian, C. A.

2012-12-01

The accumulation of dust in remote, pelagic sediments is controlled by aridity in the source regions as well as the gustiness of the transporting winds. Models and theory predict lower zonal wind intensities and gustiness in climates characterized by diminished meridional gradients such as the Late Cretaceous and Early Paleogene. The few published long-term data indicate overall lower dust accumulation in the northern Pacific and southern Indian Ocean during the Late Cretaceous and Early Paleogene than during the Neogene, as well as higher dust accumulation in the northern hemisphere than that in the south during the Late Cretaceous and Early Paleogene. However, the existing dust reconstruction likely is biased by sparse coverage, particularly from the Pacific with data limited to the northern low and subtropical latitudes. To begin examining the South Pacific, we took advantage of an extensive geochemical data set generated for DSDP Site 596, and estimated 232Th-based dust fluxes from the published 232Th concentration data and sediment mass accumulation rates. The long-term trend and absolute flux values from Site 596 are similar to that of the northern Pacific GPC3, with the exception of the late Paleocene - early Eocene and the late Neogene. We also generated a new 232Th-based dust accumulation record from IODP Site U1370 to begin examining the record from southern temperate and high latitudes (Site U1370 backtracks to close to 60°S at 50 Ma). The Site U1370 data reveal dust fluxes significantly higher than those recorded in the North Pacific, however the overall decrease from ~65 Ma to ~25 Ma is similar to the trends at Site 576 and GPC3. The new South Pacific data suggests that Sites 596 and U1370 were influenced by different prevailing winds (e.g., delivering dust from source regions with different vegetation/hydrologic conditions), different levels of storminess/gustiness, or a combination of both. If the dust fluxes recorded at Site U1370 are representative of the high latitude South Pacific, then dust supplies and storminess/gustiness in the region were higher than in the subtropics and tropics. The new dust data from Site U1370 are consistent with recent model simulations that predict higher wind intensities in the Southern Hemisphere than in the north during the early Paleogene. These results begin to suggest a significantly different reconstruction of wind gustiness, storminess and source region aridity than assumed over the past few decades.

Change Abstract Title

NASA Astrophysics Data System (ADS)

Rudich, Y.

2017-12-01

Investigating possible health effects of transported and resuspended dusts People in regions such as the Eastern Mediterranean are often exposed to high levels of both transported desert dust and to resuspended urban dust. Due to warming and drying trends, the frequency and intensity of dust storms have increased in the Eastern Mediterranean over the last decades. High exposure to particulate matter is a known risk factor to the exposed population, but the detailed understanding of how these dusts affect health remain elusive. In this talk I will describe aspects of how dust may impact health. First, transport of bacteria by desert dust, its effects on the local microbiome and dependence on the source region will be described. Then, we will describe the biological effects due to presence of biological components on dust. Finally, we will discuss how metals from brake and tire wear in resuspended urban dust affect oxidative stress and inflammation, and lead to oxidative damage in lung tissues. The significance of these findings in light of recent measurements from the global SPARATN network will be presented.

Polycyclic Aromatic Hydrocarbons in Residential Dust: Sources of Variability

PubMed Central

Metayer, Catherine; Petreas, Myrto; Does, Monique; Buffler, Patricia A.; Rappaport, Stephen M.

2013-01-01

Background: There is interest in using residential dust to estimate human exposure to environmental contaminants. Objectives: We aimed to characterize the sources of variability for polycyclic aromatic hydrocarbons (PAHs) in residential dust and provide guidance for investigators who plan to use residential dust to assess exposure to PAHs. Methods: We collected repeat dust samples from 293 households in the Northern California Childhood Leukemia Study during two sampling rounds (from 2001 through 2007 and during 2010) using household vacuum cleaners, and measured 12 PAHs using gas chromatography–mass spectrometry. We used a random- and a mixed-effects model for each PAH to apportion observed variance into four components and to identify sources of variability. Results: Median concentrations for individual PAHs ranged from 10 to 190 ng/g of dust. For each PAH, total variance was apportioned into regional variability (1–9%), intraregional between-household variability (24–48%), within-household variability over time (41–57%), and within-sample analytical variability (2–33%). Regional differences in PAH dust levels were associated with estimated ambient air concentrations of PAH. Intraregional differences between households were associated with the residential construction date and the smoking habits of residents. For some PAHs, a decreasing time trend explained a modest fraction of the within-household variability; however, most of the within-household variability was unaccounted for by our mixed-effects models. Within-household differences between sampling rounds were largest when the interval between dust sample collections was at least 6 years in duration. Conclusions: Our findings indicate that it may be feasible to use residential dust for retrospective assessment of PAH exposures in studies of health effects. PMID:23461863

Infrared dust and millimeter-wave carbon monoxide emission in the Orion region

NASA Technical Reports Server (NTRS)

Bally, John; Langer, William D.; Liu, Weihong

1991-01-01

The far-infrared dust emission seen by the IRAS satellite in the Orion region is analyzed as a function of the local radiation field intensity, and the dust temperature and opacity are compared with (C-12)O and (C-13)O emission. The infrared radiation is interpreted within the framework of a single-component large grain model and a multicomponent grain model consisting of subpopulations of grains with size-dependent temperatures. A strong dependence of the 100-micron optical depth derived is found using the large grain model on the average line-of-sight dust temperature and radiation field. In the hot environment surrounding high-luminosity sources and H II regions, all dust along the line-of-sight radiates at 100 microns, and the dust-to-gas ratio, based on the 100-micron opacity and I(/C-13/O), appears to be in agreement with the standard value, about 1 percent by mass. A relationship is found between the inferred dust-to-gas ratio and the radiation field intensity responsible for heating the dust which can be used to estimate the gas column density from the dust opacity derived from the 60- and 100-micron IRAS fluxes.

THE IMPACT OF ACCURATE EXTINCTION MEASUREMENTS FOR X-RAY SPECTRAL MODELS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Smith, Randall K.; Valencic, Lynne A.; Corrales, Lia, E-mail: lynne.a.valencic@nasa.gov

Interstellar extinction includes both absorption and scattering of photons from interstellar gas and dust grains, and it has the effect of altering a source's spectrum and its total observed intensity. However, while multiple absorption models exist, there are no useful scattering models in standard X-ray spectrum fitting tools, such as XSPEC. Nonetheless, X-ray halos, created by scattering from dust grains, are detected around even moderately absorbed sources, and the impact on an observed source spectrum can be significant, if modest, compared to direct absorption. By convolving the scattering cross section with dust models, we have created a spectral model asmore » a function of energy, type of dust, and extraction region that can be used with models of direct absorption. This will ensure that the extinction model is consistent and enable direct connections to be made between a source's X-ray spectral fits and its UV/optical extinction.« less

Seasonal and Elevational Variations of Black Carbon and Dust in Snow and Ice in the Solu-Khumbu, Nepal and Estimated Radiative Forcings

NASA Astrophysics Data System (ADS)

Kaspari, S.; Painter, T. H.; Gysel, M.; Skiles, M.; Schwikowski, M.

2014-12-01

Black carbon (BC) and dust deposited on snow and glacier surfaces can reduce the surface albedo, accelerate melt, and trigger albedo feedback. Assessing BC and dust concentrations in snow and ice in the Himalaya is of interest because this region borders large BC and dust sources, and seasonal snow and glacier ice in this region are an important source of water resources. Snow and ice samples were collected from crevasse profiles and snowpits at elevations between 5400 and 6400 m asl from Mera glacier located in the Solu-Khumbu region of Nepal. The samples were measured for Fe concentrations (used as a dust proxy) via ICP-MS, total impurity content gravimetrically, and BC concentrations using a Single Particle Soot Photometer (SP2). BC and Fe concentrations are substantially higher at elevations < 6000 m due to post-depositional processes including melt and sublimation and greater loading in the lower troposphere. Because the largest areal extent of snow and ice resides at elevations < 6000 m, the higher BC and dust concentrations at these elevations can reduce the snow and glacier albedo over large areas, accelerating melt, affecting glacier mass-balance and water resources, and contributing to a positive climate forcing. Radiative transfer modeling constrained by measurements at 5400 m at Mera La indicates that BC concentrations in the winter-spring snow/ice horizons are sufficient to reduce albedo by 6-10% relative to clean snow, corresponding to localized instantaneous radiative forcings of 75-120 W m-2. The other bulk impurity concentrations, when treated separately as dust, reduce albedo by 40-42% relative to clean snow and give localized instantaneous radiative forcings of 488 to 525 W m-2. Adding the BC absorption to the other impurities results in additional radiative forcings of 3 W m-2. While these results suggest that the snow albedo and radiative forcing effect of dust is considerably greater than BC, there are several sources of uncertainty.

SMA Continuum Survey of Circumstellar Disks in Serpens

NASA Astrophysics Data System (ADS)

Law, Charles; Ricci, Luca; Andrews, Sean M.; Wilner, David J.; Qi, Chunhua

2017-06-01

The lifetime of disks surrounding pre-main-sequence stars is closely linked to planet formation and provides information on disk dispersal mechanisms and dissipation timescales. The potential for these optically thick, gas-rich disks to form planets is critically dependent on how much dust is available to be converted into terrestrial planets and rocky cores of giant planets. For this reason, an understanding of how dust mass varies with key properties such as stellar mass, age, and environment is critical for understanding planet formation. Millimeter wavelength observations, in which the dust emission is optically thin, are required to study the colder dust residing in the disk’s outer regions and to measure disk dust masses. Hence, we have obtained SMA 1.3 mm continuum observations of 62 Class II sources with suspected circumstellar disks in the Serpens star-forming region (SFR). Relative to the well-studied Taurus SFR, Serpens allows us to probe the distribution of dust masses for disks in a much denser and more clustered environment. Only 13 disks were detected in the continuum with the SMA. We calculate the total dust masses of these disks and compare their masses to those of disks in Taurus, Lupus, and Upper Scorpius. We do not find evidence of diminished dust masses in Serpens disks relative to those in Taurus despite the fact that disks in denser clusters may be expected to contain less dust mass due to stronger and more frequent tidal interactions that can disrupt the outer regions of disks. However, considering the low detection fraction, we likely detected only bright continuum sources and a more sensitive survey of Serpens would help clarify these results.

Onset of frequent dust storms in northern China at ~AD 1100.

PubMed

He, Yuxin; Zhao, Cheng; Song, Mu; Liu, Weiguo; Chen, Fahu; Zhang, Dian; Liu, Zhonghui

2015-11-26

Dust storms in northern China strongly affect the living and health of people there and the dusts could travel a full circle of the globe in a short time. Historically, more frequent dust storms occurred during cool periods, particularly the Little Ice Age (LIA), generally attributed to the strengthened Siberian High. However, limited by chronological uncertainties in proxy records, this mechanism may not fully reveal the causes of dust storm frequency changes. Here we present a late Holocene dust record from the Qaidam Basin, where hydrological changes were previously reconstructed, and examine dust records from northern China, including the ones from historical documents. The records, being broadly consistent, indicate the onset of frequent dust storms at ~AD 1100. Further, peaked dust storm events occurred at episodes of high total solar irradiance or warm-dry conditions in source regions, superimposed on the high background of frequent dust storms within the cool LIA period. We thus suggest that besides strong wind activities, the centennial-scale dust storm events over the last 1000 years appear to be linked to the increased availability of dust source. With the anticipated global warming and deteriorating vegetation coverage, frequent occurrence of dust storms in northern China would be expected to persist.

Long-Term Variability of Airborne Asian Dust Observed from TOMS

NASA Technical Reports Server (NTRS)

Herman, J. R.; Hsu, N. C.; Seftor, C. J.; Holben, B. N.; Holben, B. N.; Einaudi, Franco (Technical Monitor)

2001-01-01

Recent studies suggest that airborne Asian dust may not only play an important role in the regional radiation budget, but also influence the air quality over North America through long-range transport. In this paper, we use satellite data to investigate the long-term variability of airborne Asian dust as well as the daily variation of the dust aerosol distribution. By combining the Total Ozone Mapping Spectrometer (TOMS) aerosol index with National Centers for Environmental Prediction (NCEP) wind data, our analysis shows a strong correlation between the generation of dust storms in the region and the passage of springtime weather fronts. This is consistent with earlier studies performed by other researchers. According to both the Nimbus-7 and Earth-Probe TOMS data the Takla Makan desert, the Gobi desert, and the and region of Inner Mongolia are major sources of the eastward-flowing airborne Asian dust. Heavily populated areas in eastern China (e.g., Beijing) are often on the primary path of the dust storms originating in these desert regions. The increasing desertification north of the Beijing region has served to exacerbate problems stemming from these storms. The time series derived from 20 years of TOMS aerosol index data shows the first significant satellite evidence of the atmospheric effect of increasing desertification, indicating that the amount of dust blown eastward has increased strongly during the past few years including the year 2000.

Evaluation of coral pathogen growth rates after exposure to atmospheric African dust samples

USGS Publications Warehouse

Lisle, John T.; Garrison, Virginia H.; Gray, Michael A.

2014-01-01

Laboratory experiments were conducted to assess if exposure to atmospheric African dust stimulates or inhibits the growth of four putative bacterial coral pathogens. Atmospheric dust was collected from a dust-source region (Mali, West Africa) and from Saharan Air Layer masses over downwind sites in the Caribbean [Trinidad and Tobago and St. Croix, U.S. Virgin Islands (USVI)]. Extracts of dust samples were used to dose laboratory-grown cultures of four putative coral pathogens: Aurantimonas coralicida (white plague type II), Serratia marcescens (white pox), Vibrio coralliilyticus, and V. shiloi (bacteria-induced bleaching). Growth of A. coralicida and V. shiloi was slightly stimulated by dust extracts from Mali and USVI, respectively, but unaffected by extracts from the other dust sources. Lag time to the start of log-growth phase was significantly shortened for A. coralicida when dosed with dust extracts from Mali and USVI. Growth of S. marcescens and V. coralliilyticus was neither stimulated nor inhibited by any of the dust extracts. This study demonstrates that constituents from atmospheric dust can alter growth of recognized coral disease pathogens under laboratory conditions.

Fine particulate matter emissions inventories: comparisons of emissions estimates with observations from recent field programs.

PubMed

Simon, Heather; Allen, David T; Wittig, Ann E

2008-02-01

Emissions inventories of fine particulate matter (PM2.5) were compared with estimates of emissions based on data emerging from U.S. Environment Protection Agency Particulate Matter Supersites and other field programs. Six source categories for PM2.5 emissions were reviewed: on-road mobile sources, nonroad mobile sources, cooking, biomass combustion, fugitive dust, and stationary sources. Ammonia emissions from all of the source categories were also examined. Regional emissions inventories of PM in the exhaust from on-road and nonroad sources were generally consistent with ambient observations, though uncertainties in some emission factors were twice as large as the emission factors. In contrast, emissions inventories of road dust were up to an order of magnitude larger than ambient observations, and estimated brake wear and tire dust emissions were half as large as ambient observations in urban areas. Although comprehensive nationwide emissions inventories of PM2.5 from cooking sources and biomass burning are not yet available, observational data in urban areas suggest that cooking sources account for approximately 5-20% of total primary emissions (excluding dust), and biomass burning sources are highly dependent on region. Finally, relatively few observational data were available to assess the accuracy of emission estimates for stationary sources. Overall, the uncertainties in primary emissions for PM2.s are substantial. Similar uncertainties exist for ammonia emissions. Because of these uncertainties, the design of PM2.5 control strategies should be based on inventories that have been refined by a combination of bottom-up and top-down methods.

Dust Aerosols at the Source Region During ACE-ASIA: A Surface/Satellite Perspective

NASA Technical Reports Server (NTRS)

Tsay, Si-Chee; Lau, William K. M. (Technical Monitor)

2001-01-01

ACE (Aerosol Characterization Experiment)-Asia is designed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentrations over eastern Asia and along the rim of the western Pacific. The phase-I of ACE-Asia was conducted from March-May 2001 in the vicinity of the Gobi desert, East Coast of China, Yellow Sea, Korea, and Japan, along the pathway of Kosa (severe events that blanket East Asia with yellow desert dust, peaked in the Spring season). Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian dust is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia we have measured continuously aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over homogeneous areas from surface. The inclusion of flux measurements permits the determination of dust aerosol radiative flux in addition to measurements of loading and optical thickness. At the time of the Terra/MODIS, SeaWiFS, TOMS and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. Preliminary results will be presented and discussed their implications in regional climatic effects.

Reddening and extinction towards H II regions

NASA Technical Reports Server (NTRS)

Caplan, James; Deharveng, Lise

1989-01-01

The light emitted by the gas in H II regions is attenuated by dust. This extinction can be measured by comparing H alpha, H beta, and radio continuum fluxes, since the intrinsic ratios of the Balmer line and thermal radio continuum emissivities are nearly constant for reasonable conditions in H II regions. In the case of giant extragalactic H II regions, the extinction was found to be considerably greater than expected. The dust between the Earth and the emitting gas may have an optical thickness which varies. The dust may be close enough to the source that scattered light contributes to the flux, or the dust may be actually mixed with the emitting gas. It is difficult to decide which configuration is correct. A rediscussion of this question in light of recent observations, with the Fabry-Perot spectrophotometers, of the large Galactic H II region is presented. The color excesses are compared for stars embedded in these H II regions with those derived (assuming the standard law) from the nebular extinction and reddening.

Cold Dust and its Heating Sources in M 33

NASA Astrophysics Data System (ADS)

Komugi, Shinya; Tosaki, Tomoka; Kohno, Kotaro; Tsukagoshi, Takashi; Tamura, Yoichi; Miura, Rie; Onodera, Sachiko; Kuno, Nario; Kawabe, Ryohei; Nakanishi, Koichiro; Sawada, Tsuyoshi; Ezawa, Hajime; Wilson, Grant W.; Yun, Min S.; Scott, Kimberly S.; Hughes, David H.; Aretxaga, Itziar; Perera, Thushara A.; Austermann, Jason E.; Tanaka, Kunihiko; Muraoka, Kazuyuki; Egusa, Fumi

2011-12-01

We have mapped the nearby face-on spiral galaxy M 33 in the 1.1 mm dust continuum using AzTEC on Atacama Submillimeter Telescope Experiment (ASTE). The preliminary results are presented here. The observed dust has a characteristic temperature of ~ 21 K in the central kpc, radially declining down to ~ 13 K at the edge of the star forming disk. We compare the dust temperatures with KS band flux and star formation tracers. Our results imply that cold dust heating may be driven by long-lived stars even nearby star forming regions.

A radiogenic isotope tracer study of transatlantic dust transport from Africa to the Caribbean

USGS Publications Warehouse

Kumar, A.; Abouchami, W.; Galer, S.J.G.; Garrison, V.H.; Williams, E.; Andreae, M.O.

2014-01-01

Many studies have suggested that long-range transport of African desert dusts across the Atlantic Ocean occurs, delivering key nutrients and contributing to fertilization of the Amazon rainforest. Here we utilize radiogenic isotope tracers – Sr, Nd and Pb – to derive the provenance, local or remote, and pathways of dust transport from Africa to the Caribbean. Atmospheric total suspended particulate (TSP) matter was collected in 2008 on quartz fibre filters, from both sides of the Atlantic Ocean at three different locations: in Mali (12.6°N, 8.0°W; 555 m a.s.l.), Tobago (11.3°N, 60.5°W; 329 m a.s.l.) and the U.S. Virgin Islands (17.7°N, 64.6°W; 27 m a.s.l.). Both the labile phase, representative of the anthropogenic signal, and the refractory detrital silicate fraction were analysed. Dust deposits and soils from around the sampling sites were measured as well to assess the potential contribution from local sources to the mineral dust collected. The contribution from anthropogenic sources of Pb was predominant in the labile, leachate phase. The overall similarity in Pb isotope signatures found in the leachates is attributed to a common African source of anthropogenic Pb, with minor inputs from other sources, such as from Central and South America. The Pb, Sr and Nd isotopic compositions in the silicate fraction were found to be systematically more radiogenic than those in the corresponding labile phases. In contrast, Nd and Sr isotopic compositions from Mali, Tobago, and the Virgin Islands are virtually identical in both leachates and residues. Comparison with existing literature data on Saharan and Sahelian sources constrains the origin of summer dust transported to the Caribbean to mainly originate from the Sahel region, with some contribution from northern Saharan sources. The source regions derived from the isotope data are consistent with 7-day back-trajectory analyses, demonstrating the usefulness of radiogenic isotopes in tracing dust provenance and atmospheric transport.

[Groups and sources of yeasts in house dust].

PubMed

Glushakova, A M; Zheltikova, T M; Chernov, I Iu

2004-01-01

House dust contains bacteria, mycelial fungi, microarthropods, and yeasts. The house dust samples collected in 25 apartments in Moscow and the Moscow region were found to contain yeasts belonging to the genera Candida, Cryptococcus, Debaryomyces, Rhodotorula, Sporobolomyces, and Trichosporon. The most frequently encountered microorganisms were typical epiphytic yeasts, such as Cryptococcus diffluens and Rhodotorula mucilaginosa, which are capable of long-term preservation in an inactive state. The direct source of epiphytic yeasts occurring in the house dust might be the indoor plants, which were contaminated with these yeasts, albeit to a lesser degree than outdoor plants. Along with the typical epiphytic yeasts, the house dust contained the opportunistic yeast pathogens Candida catenulata, C. guillermondii, C. haemulonii, C. rugosa, and C. tropicalis, which are known as the causal agents of candidiasis. We failed to reveal any correlation between the abundance of particular yeast species in the house dust, residential characteristics, and the atopic dermatitis of the inhabitants.

Hourly elemental concentrations in PM2.5 aerosols sampled simultaneously at urban background and road site during SAPUSS - diurnal variations and PMF receptor modelling

NASA Astrophysics Data System (ADS)

Dall'Osto, M.; Querol, X.; Amato, F.; Karanasiou, A.; Lucarelli, F.; Nava, S.; Calzolai, G.; Chiari, M.

2013-04-01

Hourly-resolved aerosol chemical speciation data can be a highly powerful tool to determine the source origin of atmospheric pollutants in urban environments. Aerosol mass concentrations of seventeen elements (Na, Mg, Al, S, Cl, K, Ca, Ti, V, Cr, Mn, Fe, Ni, Cu, Zn, Sr and Pb) were obtained by time (1 h) and size (PM2.5 particulate matter < 2.5 μm) resolved aerosol samples analysed by Particle Induced X-ray Emission (PIXE) measurements. In the Marie Curie European Union framework of SAPUSS (Solving Aerosol Problems by Using Synergistic Strategies), the approach used is the simultaneous sampling at two monitoring sites in Barcelona (Spain) during September-October 2010: an urban background site (UB) and a street canyon traffic road site (RS). Elements related to primary non-exhaust traffic emission (Fe, Cu), dust resuspension (Ca) and anthropogenic Cl were found enhanced at the RS, whereas industrial related trace metals (Zn, Pb, Mn) were found at higher concentrations at the more ventilated UB site. When receptor modelling was performed with positive matrix factorization (PMF), nine different aerosol sources were identified at both sites: three types of regional aerosols (regional sulphate (S) - 27%, biomass burning (K) - 5%, sea salt (Na-Mg) - 17%), three types of dust aerosols (soil dust (Al-Ti) - 17%, urban crustal dust (Ca) - 6%, and primary traffic non-exhaust brake dust (Fe-Cu) - 7%), and three types of industrial aerosol plumes-like events (shipping oil combustion (V-Ni) - 17%, industrial smelters (Zn-Mn) - 3%, and industrial combustion (Pb-Cl) - 5%, percentages presented are average source contributions to the total elemental mass measured). The validity of the PMF solution of the PIXE data is supported by very good correlations with external single particle mass spectrometry measurements. Some important conclusions can be drawn about the PM2.5 mass fraction simultaneously measured at the UB and RS sites: (1) the regional aerosol sources impact both monitoring sites at similar concentrations regardless their different ventilation conditions; (2) by contrast, local industrial aerosol plumes associated with shipping oil combustion and smelters activities have a higher impact on the more ventilated UB site; (3) a unique source of Pb-Cl (associated with combustion emissions) is found to be the major (82%) source of fine Cl in the urban agglomerate; (4) the mean diurnal variation of PM2.5 primary traffic non-exhaust brake dust (Fe-Cu) suggests that this source is mainly emitted and not resuspended, whereas PM2.5 urban dust (Ca) is found mainly resuspended by both traffic vortex and sea breeze; (5) urban dust (Ca) is found the aerosol source most affected by land wetness, reduced by a factor of eight during rainy days and suggesting that wet roads may be a solution for reducing urban dust concentrations.

Research on the Emission Inventory of Major Air Pollutants in 2012 for the Sichuan City Cluster in China

NASA Astrophysics Data System (ADS)

Qian, J.; He, Q.

2014-12-01

This paper developed a high resolution emission inventory of major pollutants in city cluster of Sichuan Basin, one of the most polluted regions in China. The city cluster included five cities, which were Chengdu, Deyang, Mianyang, Meishan and Ziyang. Pollution source census and field measurements were conducted for the major emission sources such as the industry sources, on-road mobile sources, catering sources and the dust sources. The inventory results showed that in the year of 2012, the emission of SO2、NOX、CO、PM10、PM2.5、VOCs and NH3 in the region were 143.5、251.9、1659.9、299.3、163.5、464.1 and 995kt respectively. Chengdu, the provincial capital city, had the largest emission load of every pollutant among the cities. The industry sources, including power plants, fuel combustion facilities and non-combustion processes were the largest emission sources for SO2、NOX and CO, contributing to 84%, 46.5%, 35% of total SO2, NOX and CO emissions. On-road mobile sources accounted for 46.5%, 33%, 16% of the total NOx, CO, PM2.5 emissions and 28% of the anthropogenic VOCs emission. Dust and industry sources contributed to 42% and 23% of the PM10 emission with the dust sources also as the largest source of PM2.5, contributing to 27%. Anthropogenic and biogenic sources took 75% and 25% of the total VOCs emission while 36% of anthropogenic VOCs emission was owing to solvent use. Livestock contributed to 62% of NH3 emissions, followed by nitrogen fertilizer application whose contribution was 23%. Based on the developed emission inventory and local meteorological data, the regional air quality modeling system WRF-CMAQ was applied to simulate the status of PM2.5 pollution in a regional scale. The results showed that high PM2.5 concentration was distributed over the urban area of Chengdu and Deyang. On-road mobile sources and dust sources were two major contributors to the PM2.5 pollution in Chengdu, both had an contribution ratio of 27%. In Deyang, Mianyang, Meishan and Ziyang, industry sources had a relatively high contribution ratio to the PM2.5 pollution, accounting for about 35%, 33%, 38% and 24% respectively.

Enhancement and identification of dust events in the south-west region of Iran using satellite observations

NASA Astrophysics Data System (ADS)

Taghavi, F.; Owlad, E.; Ackerman, S. A.

2017-03-01

South-west Asia including the Middle East is one of the most prone regions to dust storm events. In recent years, there was an increase in the occurrence of these environmental and meteorological phenomena. Remote sensing could serve as an applicable method to detect and also characterise these events. In this study, two dust enhancement algorithms were used to investigate the behaviour of dust events using satellite data, compare with numerical model output and other satellite products and finally validate with in-situ measurements. The results show that the use of thermal infrared algorithm enhances dust more accurately. The aerosol optical depth from MODIS and output of a Dust Regional Atmospheric Model (DREAM8b) are applied for comparing the results. Ground-based observations of synoptic stations and sun photometers are used for validating the satellite products. To find the transport direction and the locations of the dust sources and the synoptic situations during these events, model outputs (HYSPLIT and NCEP/NCAR) are presented. Comparing the results with synoptic maps and the model outputs showed that using enhancement algorithms is a more reliable way than any other MODIS products or model outputs to enhance the dust.

Potentials and problems of building detailed dust records using peat archives: An example from Store Mosse (the "Great Bog"), Sweden

NASA Astrophysics Data System (ADS)

Kylander, Malin E.; Martínez-Cortizas, Antonio; Bindler, Richard; Greenwood, Sarah L.; Mörth, Carl-Magnus; Rauch, Sebastien

2016-10-01

Mineral dust deposition is a process often overlooked in northern mid-latitudes, despite its potential effects on ecosystems. These areas are often peat-rich, providing ample material for the reconstruction of past changes in atmospheric deposition. The highly organic (up to 99% in some cases) matrix of atmospherically fed mires, however, makes studying the actual dust particles (grain size, mineralogy) challenging. Here we explore some of the potentials and problems of using geochemical data from conservative, lithogenic elements (Al, Ga, Rb, Sc, Y, Zr, Th, Ti and REE) to build detailed dust records by using an example from the 8900-yr peat sequence from Store Mosse (the ;Great Bog;), which is the largest mire complex in the boreo-nemoral region of southern Sweden. The four dust events recorded at this site were elementally distinct, suggesting different dominant mineral hosts. The oldest and longest event (6385-5300 cal yr BP) sees a clear signal of clay input but with increasing contributions of mica, feldspar and middle-REE-rich phosphate minerals over time. These clays are likely transported from a long-distance source (<100 km). While dust deposition was reduced during the second event (5300-4370 cal yr BP), this is the most distinct in terms of its source character with [Eu/Eu∗]UCC revealing the input of plagioclase feldspar from a local source, possibly active during this stormier period. The third (2380-2200 cal yr BP) and fourth (1275-1080 cal yr BP) events are much shorter in duration and the presence of clays and heavy minerals is inferred. Elemental mass accumulation rates reflect these changes in mineralogy where the relative importance of the four dust events varies by element. The broad changes in major mineral hosts, grain size, source location and approximated net dust deposition rates observed in the earlier dust events of longer duration agree well with paleoclimatic changes observed in northern Europe. The two most recent dust events are much shorter in duration, which in combination with evidence of their local and regional character, may explain why they have not been seen elsewhere.

Aerosol Optical Properties Measured Onboard the Ronald H. Brown During ACE Asia as a Function of Aerosol Chemical Composition and Source Region

NASA Technical Reports Server (NTRS)

Quinn, P. K.; Coffman, D. J.; Bates, T. S.; Welton, E. J.; Covert, D. S.; Miller, T. L.; Johnson, J. E.; Maria, S.; Russell, L.; Arimoto, R.

2004-01-01

During the ACE Asia intensive field campaign conducted in the spring of 2001 aerosol properties were measured onboard the R/V Ronald H. Brown to study the effects of the Asian aerosol on atmospheric chemistry and climate in downwind regions. Aerosol properties measured in the marine boundary layer included chemical composition; number size distribution; and light scattering, hemispheric backscattering, and absorption coefficients. In addition, optical depth and vertical profiles of aerosol 180 deg backscatter were measured. Aerosol within the ACE Asia study region was found to be a complex mixture resulting from marine, pollution, volcanic, and dust sources. Presented here as a function of air mass source region are the mass fractions of the dominant aerosol chemical components, the fraction of the scattering measured at the surface due to each component, mass scattering efficiencies of the individual components, aerosol scattering and absorption coefficients, single scattering albedo, Angstrom exponents, optical depth, and vertical profiles of aerosol extinction. All results except aerosol optical depth and the vertical profiles of aerosol extinction are reported at a relative humidity of 55 +/- 5%. An over-determined data set was collected so that measured and calculated aerosol properties could be compared, internal consistency in the data set could be assessed, and sources of uncertainty could be identified. By taking into account non-sphericity of the dust aerosol, calculated and measured aerosol mass and scattering coefficients agreed within overall experimental uncertainties. Differences between measured and calculated aerosol absorption coefficients were not within reasonable uncertainty limits, however, and may indicate the inability of Mie theory and the assumption of internally mixed homogeneous spheres to predict absorption by the ACE Asia aerosol. Mass scattering efficiencies of non-sea salt sulfate aerosol, sea salt, submicron particulate organic matter, and dust found for the ACE Asia aerosol are comparable to values estimated for ACE 1, Aerosols99, and INDOEX. Unique to the ACE Asia aerosol was the large mass fractions of dust, the dominance of dust in controlling the aerosol optical properties, and the interaction of dust with soot aerosol.

The Spatial and Seasonal Variability in Fine Mineral Dust and Coarse Mass Concentrations at Remote Sites across the United States

NASA Astrophysics Data System (ADS)

Hand, J. L.; White, W. H.; Hyslop, N. P.; Schichtel, B. A.; Gill, T. E.

2016-12-01

Mineral dust influences air quality, visibility, health, hydrology, heterogeneous chemistry, biogeochemistry, ecology, and climate. The spatial and seasonal variability of fine (PM2.5) mineral dust (FD, mineral particles with diameters less than 2.5 µm) and coarse mass (CM, mass of particles with diameters between 2.5 and 10 µm) were characterized at over 160 rural and remote sites in the United States from the Interagency Monitoring of Protected Visual Environments (IMPROVE) network. Monthly, seasonal, and annual means were computed for 2011 through 2014 to investigate the spatial and seasonal variability of FD and CM. Regions with significant FD included the Southwest in spring (≥ 50% contributions to PM2.5 mass) and in the Midwest, Midsouth, and Southeast regions in summer (20-30% of PM2.5 mass). The seasonality of FD and CM decoupled farther from local source regions suggesting long-range transport of FD or non-dust related CM. FD mineralogy was also explored and confirmed the seasonal and regional impacts of long-range transport. Temporal trends in FD from 2000-2014 revealed regions and seasons with significantly increased FD, especially the Southwest during spring months, the central United States during summer and fall, and the Southeast in summer—all regions that were associated with significant contributions of FD to PM2.5 mass. Positive trends in FD contrast negative trends in other major aerosol species over the same time periods, further enhancing the relative importance of FD to PM2.5 mass. Increased levels of FD have important implications for its environmental and climate impacts; mitigating these impacts will require identifying and characterizing source regions and causal mechanisms for dust episodes in order to better inform resource management decisions.

Remote-sensing-based analysis of landscape change in the desiccated seabed of the Aral Sea--a potential tool for assessing the hazard degree of dust and salt storms.

PubMed

Löw, F; Navratil, P; Kotte, K; Schöler, H F; Bubenzer, O

2013-10-01

With the recession of the Aral Sea in Central Asia, once the world's fourth largest lake, a huge new saline desert emerged which is nowadays called the Aralkum. Saline soils in the Aralkum are a major source for dust and salt storms in the region. The aim of this study was to analyze the spatio-temporal land cover change dynamics in the Aralkum and discuss potential implications for the recent and future dust and salt storm activity in the region. MODIS satellite time series were classified from 2000-2008 and change of land cover was quantified. The Aral Sea desiccation accelerated between 2004 and 2008. The area of sandy surfaces and salt soils, which bear the greatest dust and salt storm generation potential increased by more than 36 %. In parts of the Aralkum desalinization of soils was found to take place within 4-8 years. The implication of the ongoing regression of the Aral Sea is that the expansion of saline surfaces will continue. Knowing the spatio-temporal dynamics of both the location and the surface characteristics of the source areas for dust and salt storms allows drawing conclusions about the potential hazard degree of the dust load. The remote-sensing-based land cover assessment presented in this study could be coupled with existing knowledge on the location of source areas for an early estimation of trends in shifting dust composition. Opportunities, limits, and requirements of satellite-based land cover classification and change detection in the Aralkum are discussed.

Interactions Between Mineral Dust, Climate, and Ocean Ecosystems

NASA Technical Reports Server (NTRS)

Gasso, Santiago; Grassian, Vicki H.; Miller, Ron L.

2010-01-01

Over the past decade, technological improvements in the chemical and physical characterization of dust have provided insights into a number of phenomena that were previously unknown or poorly understood. In addition, models are now incorporating a wider range of physical processes, which will allow us to better quantify the climatic and ecological impacts of dust. For example, some models include the effect of dust on oceanic photosynthesis and thus on atmospheric CO 2 (Friedlingstein et al. 2006). The impact of long-range dust transport, with its multiple forcings and feedbacks, is a relatively new and complex area of research, where input from several disciplines is needed. So far, many of these effects have only been parameterized in models in very simple terms. For example, the representation of dust sources remains a major uncertainty in dust modeling and estimates of the global mass of airborne dust. This is a problem where Earth scientists could make an important contribution, by working with climate scientists to determine the type of environments in which easily erodible soil particles might have accumulated over time. Geologists could also help to identify the predominant mineralogical composition of dust sources, which is crucial for calculating the radiative and chemical effects of dust but is currently known for only a few regions. Understanding how climate and geological processes control source extent and characterizing the mineral content of airborne dust are two of the fascinating challenges in future dust research.

Use of MODIS Satellite Images and an Atmospheric Dust Transport Model to Evaluate Juniperus spp. Pollen Phenology and Dispersal

NASA Technical Reports Server (NTRS)

Luvall, Jeffrey C.

2011-01-01

Pollen can be transported great distances. Van de Water et. al. reported Juniperus spp. pollen was transported 200-600 km. Hence local obse rvations of plant phenology may not be consistent with the timing and source of pollen collected by pollen sampling instruments. The DREAM (Dust REgional Atmospheric Model, Nickovic et al. 2001) is a verified model for atmospheric dust transport modeling using MODIS data produ cts to identify source regions and quantities of dust. We are modifyi ng the DREAM model to incorporate pollen transport. Pollen release wi ll be estimated based on MODIS derived phenology of Juniperus spp. communities. Ground based observations records of pollen release timing and quantities will be used as verification. This information will be used to support the Centers for Disease Control and Prevention?s Nat ional Environmental Public Health Tracking Program and the State of New Mexico environmental public health decision support for asthma and allergies alerts.

Use of MODIS Satellite Images and an Atmospheric Dust Transport Model To Evaluate Juniperus spp. Pollen Phenology and Dispersal

NASA Technical Reports Server (NTRS)

Luvall, J. C.; Sprigg, W. A.; Levetin, Estelle; Huete, Alfredo; Nickovic, S.; Pejanovic, G. A.; Vukovic, A.; VandeWater, P. K.; Myers, O. B.; Budge, A. M.;

Impact of Asian Dust on Global Surface Air Quality and Radiation Budget

NASA Technical Reports Server (NTRS)

Chin, Mian; Diehl, Thomas; Yu, Hongbin; Ginoux, Paul

2006-01-01

Dust originating from Asian deserts and desertification areas can be transported regionally and globally to affect surface air quality, visibility, and radiation budget not only at immediate downwind locations (e.g., eastern Asia) but also regions far away from the sources (e.g., North America). Deposition of Asian dust to the North Pacific Ocean basin influences the ocean productivity. In this study, we will use the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model, remote sensing data form satellite and from the ground-based network, and in-situ data from aircraft and surface observations to address the following questions: - What are the effects of Asian dust on the surface air quality and visibility over Asia and North America? - What are the seasonal and spatial variations of dust deposition to the North Pacific Ocean? How does the Asian dust affect surface radiation budget?

The role of forest in mitigating the impact of atmospheric dust pollution in a mixed landscape.

PubMed

Santos, Artur; Pinho, Pedro; Munzi, Silvana; Botelho, Maria João; Palma-Oliveira, José Manuel; Branquinho, Cristina

2017-05-01

Atmospheric dust pollution, especially particulate matter below 2.5 μm, causes 3.3 million premature deaths per year worldwide. Although pollution sources are increasingly well known, the role of ecosystems in mitigating their impact is still poorly known. Our objective was to investigate the role of forests located in the surrounding of industrial and urban areas in reducing atmospheric dust pollution. This was tested using lichen transplants as biomonitors in a Mediterranean regional area with high levels of dry deposition. After a multivariate analysis, we have modeled the maximum pollution load expected for each site taking into consideration nearby pollutant sources. The difference between maximum expected pollution load and the observed values was explained by the deposition in nearby forests. Both the dust pollution and the ameliorating effect of forested areas were then mapped. The results showed that forest located nearby pollution sources plays an important role in reducing atmospheric dust pollution, highlighting their importance in the provision of the ecosystem service of air purification.

Aeolian dust in Colorado Plateau soils: Nutrient inputs and recent change in source

PubMed Central

Reynolds, Richard; Belnap, Jayne; Reheis, Marith; Lamothe, Paul; Luiszer, Fred

2001-01-01

Aeolian dust (windblown silt and clay) is an important component in arid-land ecosystems because it may contribute to soil formation and furnish essential nutrients. Few geologic surfaces, however, have been characterized with respect to dust-accumulation history and resultant nutrient enrichment. We have developed a combination of methods to identify the presence of aeolian dust in arid regions and to evaluate the roles of this dust in ecosystem processes. Unconsolidated sandy sediment on isolated surfaces in the Canyonlands region of the Colorado Plateau differs greatly in mineralogical and chemical composition from associated bedrock, mainly aeolian sandstone. Detrital magnetite in the surficial deposits produces moderately high values of magnetic susceptibility, but magnetite is absent in nearby bedrock. A component of the surficial deposits must be aeolian to account for the abundance of magnetite, which formed originally in far-distant igneous rocks. Particle-size analysis suggests that the aeolian dust component is typically as much as 20–30%. Dust inputs have enriched the sediments in many elements, including P, Mg, Na, K, and Mo, as well as Ca, at sites where bedrock lacks calcite cement. Soil-surface biologic crusts are effective dust traps that apparently record a change in dust sources over the past several decades. Some of the recently fallen dust may result from human disturbance of land surfaces that are far from the Canyonlands, such as the Mojave Desert. Some land-use practices in the study area have the potential to deplete soil fertility by means of wind-erosion removal of aeolian silt. PMID:11390965

Aeolian dust in Colorado Plateau soils: Nutrient inputs and recent change in source

USGS Publications Warehouse

Reynolds, R.; Belnap, Jayne; Lamothe, Paul; Luiszer, Fred

2001-01-01

Aeolian dust (windblown silt and clay) is an important component in arid-land ecosystems because it may contribute to soil formation and furnish essential nutrients. Few geologic surfaces, however, have been characterized with respect to dust-accumulation history and resultant nutrient enrichment. We have developed a combination of methods to identify the presence of aeolian dust in arid regions and to evaluate the roles of this dust in ecosystem processes. Unconsolidated sandy sediment on isolated surfaces in the Canyonlands region of the Colorado Plateau differs greatly in mineralogical and chemical composition from associated bedrock, mainly aeolian sandstone. Detrital magnetite in the surficial deposits produces moderately high values of magnetic susceptibility, but magnetite is absent in nearby bedrock. A component of the surficial deposits must be aeolian to account for the abundance of magnetite, which formed originally in far-distant igneous rocks. Particle-size analysis suggests that the aeolian dust component is typically as much as 20a??30%. Dust inputs have enriched the sediments in many elements, including P, Mg, Na, K, and Mo, as well as Ca, at sites where bedrock lacks calcite cement. Soil-surface biologic crusts are effective dust traps that apparently record a change in dust sources over the past several decades. Some of the recently fallen dust may result from human disturbance of land surfaces that are far from the Canyonlands, such as the Mojave Desert. Some land-use practices in the study area have the potential to deplete soil fertility by means of wind-erosion removal of aeolian silt.

Geochemical fingerprint of desert surface sediments and aeolian dust exported from southern South America

NASA Astrophysics Data System (ADS)

Gili, S.; Gaiero, D. M.; Jweda, J.; Koestner, E.; Chemale, F.; Kaplan, M. R.; Goldstein, S. L.

2012-12-01

Wind-transported dust is a tracer of atmospheric circulation and also provides important information about the climatic conditions prevailing in dust source areas. Understanding the origin of mineral dust deposited in different environments (e.g., continent, ocean, polar ice sheet) and the variability of its concentration and composition, can be used as a proxy for the interpretation of the wind systems characteristics and probable changes in the atmospheric circulation patterns. In order to improve the atmospheric circulation models developed for the Southern Hemisphere, it is necessary to increase the understanding of the characteristics of the South American dust sources. Prospero et al., (2002), showed the existence of three present-day persist dust sources in South America: Patagonia (39°-52°S), central-western Argentina (26°-33°S), and the Puna-Altiplano plateau (19°-26°S). An important question to be addressed is whether these dust sources were also important during the last glacial-interglacial cycles. In most cases, researchers working in the reconstruction of paleo-environments in the Southern Hemisphere have employed sparse geochemical and isotopic data from southern South American samples. As a consequence, there are no regional or systematic studies that define their geochemical "fingerprints" of likely sources. The main goal of this work is to identify the "fingerprints" of materials exported from these areas by means of rare earth elements (REEs) and Sr-Nd-Pb-isotopes measured in surface sediments (topsoils) and mineral dust samples. Samples (n=86) were taken across the "arid diagonal" of southern South America in a N-S transect from Uyuni (20°39'S, 68°11'W, Bolivia) to Bahia Blanca (38°43'S, 62°15'W, Argentina) representing different geomorphologic environments: e.g., ephemeral lakes, lowland areas, edges of salt flats, alluvial fans, dunes, etc. Preliminary data indicate the existence of a heterogeneous chemical/isotopic signature along the "arid diagonal": a) the Altiplano and Puna have chemical and isotopic compositions inherited from the large volume of Cenozoic ignimbrites and from the Late Paleozoic granitoids (south of 21°S), respectively, b) the potential dust source in central-western Argentina appears to show a separate geochemical fingerprint explained basically by the mixing of metamorphic rocks from Eastern Sierras Pampeanas, Central Argentina and, c) dust from Patagonia with clear chemical/isotopic signatures characteristic of the Quaternary volcanism (Gaiero et al., 2004; 2007). These results are promising, as they would enable the identification of the main dust source regions in provenance studies of different paleoclimatic records (Pampean loess, Antarctic ice cores, Atlantic and Southern oceans, etc).

Dusty cradles in a turbulent nursery: the SGR A east H II region complex at the galactic center

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lau, R. M.; Herter, T. L.; Adams, J. D.

2014-10-20

We present imaging at 19, 25, 31, and 37 μm of the compact H II region complex G-0.02-0.07 located 6 pc in projection from the center of the Galaxy obtained with SOFIA using FORCAST. G-0.02-0.07 contains three compact H II regions (A, B, and C) and one ultra-compact H II region (D). Our observations reveal the presence of two faint, infrared sources located 23'' and 35'' to the east of region C (FIRS 1 and 2) and detect dust emission in two of the three 'ridges' of ionized gas west of region A. The 19/37 color temperature and 37 μmmore » optical depth maps of regions A-C are used to characterize the dust energetics and morphology. Regions A and B exhibit average 19/37 color temperatures of ∼105 K, and regions C and D exhibit color temperatures of ∼115 K and ∼130 K, respectively. Using the DustEM code, we model the SEDs of regions A-D and FIRS 1, all of which require populations of very small, transiently heated grains and large, equilibrium-heated grains. We also require the presence of polycyclic aromatic hydrocarbons in regions A-C in order to fit the 3.6, 4.5, 5.8, and 8.0 μm fluxes observed by Spitzer/IRAC. The location of the heating source for region A is determined by triangulation from distances and temperatures derived from DustEM models fit to SEDs of three different points around the region, and it is found to be displaced to the northeast of the center of curvature near the color temperature peak. Based on total luminosity, expected 1.90 μm fluxes, and proximity to the mid-IR color temperature peaks, we identify heating source candidates for regions A, B, and C. However, for region D, the observed fluxes at 1.87 and 1.90 μm of the previously proposed ionizing star are a factor of ∼40 times too bright to be the heating source and hence is likely just a star lying along the line of sight toward region D.« less

Atmospheric Dust Modeling from Meso to Global Scales with the Online NMMB/BSC-Dust Model Part 2: Experimental Campaigns in Northern Africa

NASA Technical Reports Server (NTRS)

Haustein, K.; Perez, C.; Baldasano, J. M.; Jorba, O.; Basart, S.; Miller, R. L.; Janjic, Z.; Black, T.; Nickovic, S.; Todd, M. C.;

Long-term variability of dust optical depths on Mars during MY24-MY32 and their impact on subtropical lower ionosphere: Climatology, modeling, and observations

NASA Astrophysics Data System (ADS)

Sheel, Varun; Haider, S. A.

2016-08-01

Dust optical depths (τ) for nine Martian years (MY24-MY32) in the subtropical region (25-35°S) have been used to classify distinct dust scenarios. These data are based on observations at 9.3 µm from the Mars Global Surveyor and Mars Odyssey missions and encompass the regional dust storms which occur every year around solar longitude (Ls) ~ 220° and the two major dust storms of MY25 and MY28. Constrained by these observations and the Mars Climate Sounder observations of detached dust layers, we estimate altitude profiles of dust concentrations. We discuss the characteristics of dust aerosol particles of different size between 0.2 and 3.0 µm by assuming a modified gamma distribution. We then use a comprehensive ion-dust model to calculate ion densities and conductivities in the lower ionosphere of Mars in the absence of dust storm at τ = 0.1 and Ls = 150° and for three dust storm periods viz., (1) major dust storm at τ = 1.7 and Ls = 210°, (2) major dust storm at τ = 1.2 and Ls = 280°, and (3) regional dust storm at τ = 0.5 and Ls = 220°. The model with 12 neutral species considers galactic cosmic rays as a source of ionization. Results show that the density of the dominant hydrated cluster ions and the electrical conductivity are reduced by an order of magnitude near the surface for a few months until the dust storm settles down to its normal condition.

Geochemical and microbiological fingerprinting of airborne dust that fell in Canberra, Australia, in October 2002

NASA Astrophysics Data System (ADS)

de Deckker, Patrick; Abed, Raeid M. M.; de Beer, Dirk; Hinrichs, Kai-Uwe; O'Loingsigh, Tadhg; Schefuß, Enno; Stuut, Jan-Berend W.; Tapper, Nigel J.; van der Kaars, Sander

2008-12-01

During the night of 22-23 October 2002, a large amount of airborne dust fell with rain over Canberra, located some 200 km from Australia's east coast, and at an average altitude of 650 m. It is estimated that during that night about 6 g m-2 of aeolian dust fell. We have conducted a vast number of analyses to "fingerprint" some of the dust and used the following techniques: grain size analysis; scanning electron microscope imagery; major, trace, and rare earth elemental, plus Sr and Nd isotopic analyses; organic compound analyses with respective compound-specific isotope analyses; pollen extraction to identify the vegetation sources; and molecular cloning of 16S rRNA genes in order to identify dust bacterial composition. DNA analyses show that most obtained 16S rRNA sequences belong mainly to three groups: Proteobacteria (25%), Bacteriodetes (23%), and gram-positive bacteria (23%). In addition, we investigated the meteorological conditions that led to the dust mobilization and transport using model and satellite data. Grain sizes of the mineral dust show a bimodal distribution typical of proximal dust, rather than what is found over oceans, and the bimodal aspect of size distribution confirms wet deposition by rain droplets. The inorganic geochemistry points to a source along/near the Darling River in NW New South Wales, a region that is characteristically semiarid, and both the organic chemistry and palynoflora of the dust confirm the location of this source area. Meteorological reconstructions of the event again clearly identify the area near Bourke-Cobar as being the source of the dust. This study paves the way for determining the export of Australian airborne dust both in the oceans and other continents.

Assessments of the contribution of land use change to the dust emission in Central Asia

NASA Astrophysics Data System (ADS)

Xi, X.; Sokolik, I. N.

2015-12-01

While the dust emission from arid and semi-arid regions is known as a natural process induced by wind erosion, human may affect the dust emission directly through land use disturbances and indirectly by climate change. There has been much debate on the relative importance of climate change and land use to the global dust budget, as past estimates on the proportion of dust contributed by land use, in particular agricultural practices, remains very uncertain. This to the large extent stems from the way how human-made dust sources are identified and how they are treated in models. This study attempts to assess the land use contribution to the dust emission in Central Asia during 2000-2014 by conducting multiple experiments on the total emission in the WRF-Chem-DuMo model, and applying two methods to separate the natural and anthropogenic sources. The model experiments include realistic treatments of agriculture (e.g., expansion and abandonment) and water body changes (e.g., Aral Sea desiccation) in the land cover map of WRF-Chem-DuMo, but impose no arbitrary labeling of dust source type or adjustment to the erosion threshold. Intercomparison of the model experiments will be focused on the magnitude, interannual variability, and climate sensitivity of dust fluxes resulting from the selections of surface input data and dust flux parameterizations. Based on annual land use intensity maps, the sensitivity of the anthropogenic dust proportion to selection of the threshold value will be evaluated. In conjunction with the empirical method, satellite-derived annual land classifications will be used to track the land cover dynamics, and separate potential human-made source areas.

Trans-Pacific transport of dust aerosols from East Asia: Insights gained from multiple observations and modeling.

PubMed

Guo, Jianping; Lou, Mengyun; Miao, Yucong; Wang, Yuan; Zeng, Zhaoliang; Liu, Huan; He, Jing; Xu, Hui; Wang, Fu; Min, Min; Zhai, Panmao

2017-11-01

East Asia is one of the world's largest sources of dust and anthropogenic pollution. Dust particles originating from East Asia have been recognized to travel across the Pacific to North America and beyond, thereby affecting the radiation incident on the surface as well as clouds aloft in the atmosphere. In this study, integrated analyses are performed focusing on one trans-Pacific dust episode during 12-22 March 2015, based on space-borne, ground-based observations, reanalysis data combined with Hybrid Single Particle Lagrangian Integrated Trajectory Model (HYSPLIT), and the Weather Research and Forecasting Model coupled with Chemistry (WRF-Chem). From the perspective of synoptic patterns, the location and strength of Aleutian low pressure system largely determined the eastward transport of dust plumes towards western North America. Multi-sensor satellite observations reveal that dust aerosols in this episode originated from the Taklimakan and Gobi Deserts. Moreover, the satellite observations suggest that the dust particles can be transformed to polluted particles over the East Asian regions after encountering high concentration of anthropogenic pollutants. In terms of the vertical distribution of polluted dust particles, at the very beginning, they were mainly located in the altitudes ranging from 1 km to 7 km over the source region, then ascended to 2 km-9 km over the Pacific Ocean. The simulations confirm that these elevated dust particles in the lower free troposphere were largely transported along the prevailing westerly jet stream. Overall, observations and modeling demonstrate how a typical springtime dust episode develops and how the dust particles travel over the North Pacific Ocean all the way to North America. Copyright © 2017 Elsevier Ltd. All rights reserved.

Source analysis of radiocesium in river waters using road dust tracers.

PubMed

Murakami, Michio; Saha, Mahua; Iwasaki, Yuichi; Yamashita, Rei; Koibuchi, Yukio; Tsukada, Hirofumi; Takada, Hideshige; Sueki, Keisuke; Yasutaka, Tetsuo

2017-11-01

Following the Fukushima Dai-ichi Nuclear Power Station accident, regional road dust, heavily contaminated with radiocesium, now represents a potential source of radiocesium pollution in river water. To promote effective countermeasures for reducing the risk from radiocesium pollution, it is important to understand its sources. This study evaluated the utility of metals, including Al, Fe, and Zn as road dust tracers, and applied them to analyze sources of 137 Cs in rivers around Fukushima during wet weather. Concentrations of Zn in road dust were higher than agricultural and forest soils, whereas concentrations of Fe and Al were the opposite. Concentrations of Zn were weakly but significantly correlated with benzothiazole, a molecular marker of tires, indicating Zn represents an effective tracer of road dust. Al, Fe, and Zn were frequently detected in suspended solids in river water during wet weather. Distribution coefficients of these metals and 137 Cs exceeded 10 4 , suggesting sorptive behavior in water. Although concentrations of Al, Fe, Zn, and 137 Cs were higher in fine fractions of road dust and soils than in coarse fractions, use of ratios of 137 Cs to Al, Fe, or Zn showed smaller differences among size fractions. The results demonstrate that combinations of these metals and 137 Cs are useful for analyzing sources of radiocesium in water. These ratios in river water during wet weather were found to be comparable with or lower than during dry weather and were closer to soils than road dust, suggesting a limited contribution from road dust to radiocesium pollution in river water. Copyright © 2017 Elsevier Ltd. All rights reserved.

MISR Decadal Observations of Mineral Dust: Property Characterization and Climate Applications

NASA Technical Reports Server (NTRS)

Kalashnikova, Olga V.; Garay, Michael J.; Sokolik, Irina; Kahn, Ralph A.; Lyapustin, A.; Diner, David J.; Lee, Jae N.; Torres, Omar; Leptoukh, Gregory G.; Sabbah, Ismail

2012-01-01

The Multi-angle Imaging SpectroRadiometer (MISR) provides a unique, independent source of data for studying dust emission and transport. MISR's multiple view angles allow the retrieval of aerosol properties over bright surfaces, and such retrievals have been shown to be sensitive to the non-sphericity of dust aerosols over both land and water. MISR stereographic views of thick aerosol plumes allow height and instantaneous wind derivations at spatial resolutions of better than 1.1 km horizontally and 200m vertically. We will discuss the radiometric and stereo-retrieval capabilities of MISR specifically for dust, and demonstrate the use of MISR data in conjunction with other available satellite observations for dust property characterization and climate studies.First, we will discuss MISR non-spherical (dust) fraction product over the global oceans. We will show that over the Atlantic Ocean, changes in the MISR-derived non-spherical AOD fraction illustrate the evolution of dust during transport. Next, we will present a MISR satellite perspective on dust climatology in major dust source regions with a particular emphasis on the West Africa and Middle East and discuss MISR's unique strengths as well as current product biases. Finally, we will discuss MISR dust plume product and climatological applications.

Modeling the biogeochemical impact of atmospheric phosphate deposition from desert dust and combustion sources to the Mediterranean Sea

NASA Astrophysics Data System (ADS)

Richon, Camille; Dutay, Jean-Claude; Dulac, François; Wang, Rong; Balkanski, Yves

2018-04-01

Daily modeled fields of phosphate deposition to the Mediterranean from natural dust, anthropogenic combustion and wildfires were used to assess the effect of this external nutrient on marine biogeochemistry. The ocean model used is a high-resolution (1/12°) regional coupled dynamical-biogeochemical model of the Mediterranean Sea (NEMO-MED12/PISCES). The input fields of phosphorus are for 2005, which are the only available daily resolved deposition fields from the global atmospheric chemical transport model LMDz-INCA. Traditionally, dust has been suggested to be the main atmospheric source of phosphorus, but the LMDz-INCA model suggests that combustion is dominant over natural dust as an atmospheric source of phosphate (PO4, the bioavailable form of phosphorus in seawater) for the Mediterranean Sea. According to the atmospheric transport model, phosphate deposition from combustion (Pcomb) brings on average 40.5×10-6 mol PO4 m-2 yr-1 over the entire Mediterranean Sea for the year 2005 and is the primary source over the northern part (e.g., 101×10-6 mol PO4 m-2 yr-1 from combustion deposited in 2005 over the north Adriatic against 12.4×10-6 from dust). Lithogenic dust brings 17.2×10-6 mol PO4 m-2 yr-1 on average over the Mediterranean Sea in 2005 and is the primary source of atmospheric phosphate to the southern Mediterranean Basin in our simulations (e.g., 31.8×10-6 mol PO4 m-2 yr-1 from dust deposited in 2005 on average over the south Ionian basin against 12.4×10-6 from combustion). The evaluation of monthly averaged deposition flux variability of Pdust and Pcomb for the 1997-2012 period indicates that these conclusions may hold true for different years. We examine separately the two atmospheric phosphate sources and their respective flux variability and evaluate their impacts on marine surface biogeochemistry (phosphate concentration, chlorophyll a, primary production). The impacts of the different phosphate deposition sources on the biogeochemistry of the Mediterranean are found localized, seasonally varying and small, but yet statistically significant. Differences in the geographical deposition patterns between phosphate from dust and from combustion will cause contrasted and significant changes in the biogeochemistry of the basin. We contrast the effects of combustion in the northern basin (Pcomb deposition effects are found to be 10 times more important in the northern Adriatic, close to the main source region) to the effects of dust in the southern basin. These different phosphorus sources should therefore be accounted for in modeling studies.

Simulating the Regional Impact of Dust on the Middle East Climate and the Red Sea

NASA Astrophysics Data System (ADS)

Osipov, Sergey; Stenchikov, Georgiy

2018-02-01

The Red Sea is located between North Africa and the Arabian Peninsula, the largest sources of dust in the world. Satellite retrievals show very high aerosol optical depth in the region, which increases during the summer season, especially over the southern Red Sea. Previously estimated and validated radiative effect from dust is expected to have a profound thermal and dynamic impact on the Red Sea, but that impact has not yet been studied or evaluated. Due to the strong dust radiative effect at the sea surface, uncoupled ocean modeling approaches with prescribed atmospheric boundary conditions result in an unrealistic ocean response. Therefore, to study the impact of dust on the regional climate of the Middle East and the Red Sea, we employed the Regional Ocean Modeling System fully coupled with the Weather Research and Forecasting model. We modified the atmospheric model to account for the radiative effect of dust. The simulations show that, in the equilibrium response, dust cools the Red Sea, reduces the surface wind speed, and weakens both the exchange at the Bab-el-Mandeb strait and the overturning circulation. The salinity distribution, freshwater, and heat budgets are significantly altered. A validation of the simulations against satellite products indicates that accounting for radiative effect from dust almost completely removes the bias and reduces errors in the top of the atmosphere fluxes and sea surface temperature. Our results suggest that dust plays an important role in the energy balance, thermal, and circulation regimes in the Red Sea.

Do Sahara dunes make dust? Some dunes do and some dunes don't

NASA Astrophysics Data System (ADS)

Bristow, Charlie

2017-04-01

The Sahara desert is responsible for producing around half of the atmospheric mineral dust on Earth. While most of the Sahara has the potential to produce dust some areas have been identified using remote sensing as especially prolific dust sources such as the Bodélé Depression in Chad which is described as the dustiest place on Earth. Geomorphological analysis indicates that these areas are usually topographic lows, such as the Bodélé, as well as regions on the flanks of topographic highs. This view was challenged by Crouvi et al. (2012) who suggest that active sand dunes are the most frequent dust sources. In this paper we use an experimental dust chamber to generate dust from dune sediments collected from the crest of active sand dunes across the Sahara including samples from the Bodélé depression, as well as dune sands from Algeria, Egypt, Libya, Morocco and Tunisia. The experiments produced a wide range of results indicating that some dune sands, including those from the Bodélé produce much more dust than others.

Natural and Anthropogenic Aerosols in the World's Megacities and Climate Impacts

NASA Astrophysics Data System (ADS)

Kafatos, M.; Singh, R.; El-Askary, H.; Qu, J.

2005-12-01

The world's megacities are the sites of production of a variety of aerosols and are themselves affected by natural and human-induced aerosols. In particular, sources of aerosols impacting cities include: industrial and automobile emission; sand and dust storms from, e.g., the Sahara and Gobi Deserts; as well as fire-induced aerosols. Improving the ability of various stakeholder organizations to respond effectively to high concentrations of aerosols, with special emphasis on mineral dust from dust storms; smoke from controlled burns, wild fires and agricultural burning; and anthropogenic aerosols, would be an important goal not just to understand climate forcings but also to be able to better respond to the increasing amounts of aerosols at global and regional levels. Cities and surrounding areas are affected without good estimates of the current and future conditions of the aerosols and their impact on regional and global climate. Remotely sensed (RS) NASA, NOAA and international platform data can be used to characterize the properties of aerosol clouds and special hazard events such as sand and dust storms (SDS). Aerosol analysis and prediction-model capabilities from which stakeholders can choose the tools that best match their needs and technological expertise are important. Scientists validating mesoscale and aerosol-transport models, aerosol retrievals from satellite measurements are indispensable for robust climate predictions. Here we give two examples of generic SDS cases and urban pollution and their possible impact on climate: The Sahara desert is a major source of dust aerosols dust transport is an important climatic process. The aerosols in the form of dust particles reflect the incoming solar radiation to space, thereby reducing the amount of radiation available to the ground, known as `direct' radiative forcing of aerosols. The aerosols also change the cloud albedo and microphysical properties of clouds, known as `indirect' radiative forcing of aerosols. The highest boundary layer heights are associated with regions where the sensible heat flux is greatest, and latent heat flux is smallest due to lack of vegetation. Boundary layer heights in the deserts may be systematically higher than the slightly wetter regions at the edges of deserts. Latent heat flux model runs and MODIS observations of dust storms affecting the Nile Delta and Cairo indicate strong influence on the local weather and climate forcings. In the Indo-Gangetic, during the pre-monsoon period, dust storms form. We have examined SDS transport using RS data acquired from NASA's MODIS MISR instruments and from sun photometer measurements. The aerosol optical depth and size of the dust particles are found to be significantly higher during such dust storm events. Moreover, our results clearly show that power plants in this region are the key point source of air pollutants. The detailed analysis of aerosol parameters show the existence of absorbing and non-absorbing aerosols emitted from these plants. The combined effects of urban aerosols with dust aerosols in India and Cairo not only affect megacities, they also have long-term climate impacts. We will also discuss how the assimilation of RS data into mesoscale models can improve these models and predictability of hazards and effects on megacities, such as SDS events, and forest fires, all sources of aerosols. Therefore RS data can improve the prediction of climate forcings by aerosols.

Threshold friction velocity influenced by wetness of soils within the Columbia Plateau

USDA-ARS?s Scientific Manuscript database

Windblown dust impacts air quality in the Columbia Plateau of the U.S. Pacific Northwest. Wind erosion of agricultural lands, which is the predominate source of windblown dust in the region, occurs when the friction velocity exceeds the threshold friction velocity (TFV) of the surface. Soil moisture...

Study of Chinese pollution with the 3D regional chemistry transport CHIMERE model and remote sensing observations, with a focus on mineral dust impacts

NASA Astrophysics Data System (ADS)

Lachatre, Mathieu; Foret, Gilles; Beekmann, Matthias; Cheiney, Audrey; Dufour, Gaëlle; Laurent, Benoit; Cuesta, Juan

2017-04-01

Since the end of the 20th century, China has observed important growth in numerous sectors. China's Gross Domestic Product (GDP) has been multiply by 4 during the 2000-2010 decade (National Bureau of Statistics of China), mostly because of the industry's growth. These evolutions have been accompanied by important increases of atmospheric pollutants emissions (Yinmin et al, Atmo Env, 2016). As a consequence and for about 10 years now, Chinese authorities have been working to reduce pollutant levels, because atmospheric pollution is a major health issue for Chinese population especially within cities, for which World Health Organisation's standards for major pollutants (Ozone, PM2.5, PM10) are often exceeded. Particles have multiple issues, as they impact on health and global warming. Their impacts will depend on their sources (primary or secondary pollutants) and natures (Particle size distribution, chemical composition…). Controlling particles loading is a complex task as their sources are various and dispersed on the Chinese territories: mineral dust can be emitted from Chinese deserts in large amount (Laurent et al., GPC, 2006), ammonia can be emitted from agriculture and livestock (Kang et al., ACP, 2016) and lots of urban primary pollutants can be emitted from urbanized areas. It is then necessary to work from a continental to local scales to understand more precisely pollution of urbanized areas. It is then mandatory to discriminate and quantify pollution sources and to estimate the impact of natural pollution and the major contributing sources. We propose here an approach based on a model and satellite observation synergy to estimate what controls Chinese pollution. We use the regional chemistry transport model CHIMERE (Menut et al., GMD, 2013) to simulate atmospheric pollutants concentrations. A large domain (72°E-145°E; 17.5°N-55°N), with a ¼°x¼° resolution is used to make multi-annual simulations. CHIMERE model include most of the pollutants sources, and using a soil properties database is able to model Dust emissions (Laurent B. et al., JGR, 2005). Satellite products are available to evaluate and improve our simulations, as for example the AOD and Angstrom coefficient from the MODIS instrument. Mineral dust pollution represents one of the most important sources of atmospheric pollutant over Chinese territories, but dust emissions and transport present important seasonal variabilities. To evaluate impacts of dust pollutants on inhabited areas' pollutions, we compute dust emissions (Marticorena and Bergametti, JGR, 1995) and transport. Using MODIS instrument information over dust source regions, we control that AOD amplitudes and temporal variations simulated with CHIMERE correspond. We attempt to quantify the impact of mineral dust pollution each month over several urbanized areas using multi-annual simulations (2011, 2013, and 2015). We also investigate the impact of heavy dust events within inhabited areas' pollution. This work is also part of the French funded project "Pollution in Eastern Asia: towards better air quality prevision and impacts' evaluation".

Long-term Satellite Observations of Asian Dust Storm: Source, Pathway, and Interannual Variability

NASA Technical Reports Server (NTRS)

Hsu, N. Christina

2008-01-01

Among the many components that contribute to air pollution, airborne mineral dust plays an important role due to its biogeochemical impact on the ecosystem and its radiative-forcing effect on the climate system. In East Asia, dust storms frequently accompany the cold and dry air masses that occur as part of springtime cold front systems. Outbreaks of Asian dust storms occur often in the arid and semi-arid areas of northwestern China -about 1.6x10(exp 6) square kilometers including the Gobi and Taklimakan deserts- with continuous expanding of spatial coverage. These airborne dust particles, originating in desert areas far from polluted regions, interact with anthropogenic sulfate and soot aerosols emitted from Chinese megacities during their transport over the mainland. Adding the intricate effects of clouds and marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from their sources. Furthermore, these aerosols, once generated over the source regions, can be transported out of the boundary layer into the free troposphere and can travel thousands of kilometers across the Pacific into the United States and beyond. In this paper, we will demonstrate the capability of a new satellite algorithm to retrieve aerosol properties (e.g., optical thickness, single scattering albedo) over bright-reflecting surfaces such as urban areas and deserts. Such retrievals have been difficult to perform using previously available algorithms that use wavelengths from the mid-visible to the near IR because they have trouble separating the aerosol signal from the contribution due to the bright surface reflectance. This new algorithm, called Deep Blue, utilizes blue-wavelength measurements from instruments such as SeaWiFS and MODIS to infer the properties of aerosols, since the surface reflectance over land in the blue part of the spectrum is much lower than for longer wavelength channels. Reasonable agreements have been achieved between Deep Blue retrievals of aerosol optical thickness and those directly from AERONET sunphotometers over desert and semi-desert regions. New Deep Blue products will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from SeaWiFS and MODIS-like instruments. Long-term satellite measurements (1998 - 2007) from SeaWiFS will be utilized to investigate the interannual variability of source, pathway, and dust loading associated with the Asian dust storm outbreaks. In addition, monthly averaged aerosol optical thickness during the springtime from SeaWiFS will also be compared with the MODIS Deep Blue products.

An assessment of SEVIRI imagery at different temporal resolutions and the effect on accurate dust emission mapping

NASA Astrophysics Data System (ADS)

Hennen, Mark; White, Kevin; Shahgedanova, Maria

2017-04-01

This paper compares Dust RGB products derived from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) data at 15 minute, 30 minute and hourly temporal resolutions. From January 2006 to December 2006, observations of dust emission point sources were observed at each temporal resolution across the entire Middle East region (38.50N; 30.00E - 10.00N; 65.50E). Previous work has demonstrated that 15-minute resolution SEVIRI data can be used to map dust sources across the Sahara by observing dust storms back through sequential images to the point of first emission (Schepanski et al., 2007; 2009; 2012). These observations have improved upon lower resolution maps, based on daily retrievals of aerosol optical depth (AOD), whose maxima can be biased by prevalent transport routes, not necessarily coinciding with sources of emissions. Based on the thermal contrast of atmospheric dust to the surface, brightness temperature differences (BTD's) in the thermal infrared (TIR) wavelengths (8.7, 10.8 and 12.0 µm) highlight dust in the scene irrespective of solar illumination, giving both increased accuracy of dust source areas and a greater understanding of diurnal emission behaviour. However, the highest temporal resolution available (15-minute repeat capture) produces 96 images per day, resulting in significantly higher data storage demands than 30 minute or hourly data. To aid future research planning, this paper investigates what effect lowering the temporal resolution has on the number and spatial distribution of the observed dust sources. The results show a reduction in number of dust emission events observed with each step decrease in temporal resolution, reducing by 17% for 30-minute resolution and 50% for hourly. These differences change seasonally, with the highest reduction observed in summer (34% and 64% reduction respectively). Each resolution shows a similar spatial distribution, with the biggest difference seen near the coastlines, where near-shore convective cloud patterns obscure atmospheric dust soon after emission, restricting the opportunity to be observed at hourly resolution.

On the dust load and rainfall relationship in South Asia: an analysis from CMIP5

NASA Astrophysics Data System (ADS)

Singh, Charu; Ganguly, Dilip; Dash, S. K.

2018-01-01

This study is aimed at examining the consistency of the relationship between load of dust and rainfall simulated by different climate models and its implication for the Indian summer monsoon system. Monthly mean outputs of 12 climate models, obtained from the archive of the Coupled Model Intercomparison Project phase 5 (CMIP5) for the period 1951-2004, are analyzed to investigate the relationship between dust and rainfall. Comparative analysis of the model simulated precipitation with the India Meteorological Department (IMD) gridded rainfall, CRU TS3.21 and GPCP version 2.2 data sets show significant differences between the spatial patterns of JJAS rainfall as well as annual cycle of rainfall simulated by various models and observations. Similarly, significant inter-model differences are also noted in the simulation of load of dust, nevertheless it is further noted that most of the CMIP5 models are able to capture the major dust sources across the study region. Although the scatter plot analysis and the lead-lag pattern correlation between the dust load and the rainfall show strong relationship between the dust load over distant sources and the rainfall in the South Asian region in individual models, the temporal scale of this association indicates large differences amongst the models. Our results caution that it would be pre-mature to draw any robust conclusions on the time scale of the relationship between dust and the rainfall in the South Asian region based on either CMIP5 results or limited number of previous studies. Hence, we would like to emphasize upon the fact that any conclusions drawn on the relationship between the dust load and the South Asian rainfall using model simulation is highly dependent on the degree of complexity incorporated in those models such as the representation of aerosol life cycle, their interaction with clouds, precipitation and other components of the climate system.

Use of dust storm observations on satellite images to identify areas vulnerable to severe wind erosion

USGS Publications Warehouse

Breed, C.S.; McCauley, J.F.

1986-01-01

Blowing dust is symptomatic of severe wind erosion and deterioration of soils in areas undergoing dessication and/or devegetation. Dust plumes on satellite images can commonly be traced to sources in marginally arable semiarid areas where protective lag gravels or vegetation have been removed and soils are dry, as demonstrated for the Portales Valley, New Mexico. Images from Landsat and manned orbiters such as Skylab and the Space Shuttle are useful for illustrating the regional relations of airborne dust plumes to source areas. Geostationary satellites such as GOES are useful in tracking the time-histories of episodic dust storms. These events sometimes go unrecognized by weather observers and are the precursors of long-term land degradation trends. In areas where soil maps and meteorological data are inadequate, satellite images provide a means for identifying problem areas where measures are needed to control or mitigate wind erosion. ?? 1986 D. Reidel Publishing Company.

Modeling of intercontinental Saharan dust transport: What consequences on atmospheric concentrations and deposition fluxes in the Caribbean?

NASA Astrophysics Data System (ADS)

Laurent, Benoit; Formenti, Paola; Desboeufs, Karine; Vincent, Julie; Denjean, Cyrielle; Siour, Guillaume; Mayol-Bracero, Olga L.

2015-04-01

The Dust Aging and Transport from Africa to the Caribbean (Dust-AttaCk) project aims todocument the physical and optical properties of long-range transported African dust to the Caribbean. A comprehensive field campaign was conducted in Cape San Juan, Puerto Rico (18.38°N 65.62°W) during June-July 2012, offering the opportunity to constrain the way Saharan dust are transported from North Africa to the Caribbean by 3D models. Our main objectives are: (i) to discuss the ability of the CHIMERE Eulerian off-line chemistry-transport model to simulate atmospheric Saharan dust loads observed in the Caribbean during the Dust-AttaCk campaign, as well as the altitude of the dust plumes transport over the North Atlantic Ocean up to the Caribbean, (ii) to study the main Saharan dust emission source areas contributing to the dust loads in the Caribbean, (iii) to estimate the Saharan dust deposition in the Caribbean for deposition events observed during the Dust-AttaCk campaign. The dust model outputs are hourly dust concentration fields in µg m-3 for 12 aerosol size bins up to 30 µm and for each of the 15 sigma pressure vertical levels, column integrated dustaerosol optical depth (AOD), and dry and wet deposition fluxes.The simulations performed for the Dust-AttaCk campaign period as well as satellite observations (MODIS AOD, SEVIRI AOD) are used to identify the Saharan emission source regions activated and to study the evolution of the dust plumes tothe Cape San Juan station. In complement, the vertical transport of dust plumes transported from Saharan dust sources and over the North Atlantic Ocean is investigated combining model simulations and CALIOP observations. Aerosol surface concentrations and AOD simulated with CHIMERE are compared with sin-situ observations at Cape San Juan and AERONET stations. Wet deposition measurements performed allow us to constrain dust deposition flux simulated in the Caribbean after long-range transport.

Quantifying global dust devil occurrence from meteorological analyses

PubMed Central

Jemmett-Smith, Bradley C; Marsham, John H; Knippertz, Peter; Gilkeson, Carl A

2015-01-01

Dust devils and nonrotating dusty plumes are effective uplift mechanisms for fine particles, but their contribution to the global dust budget is uncertain. By applying known bulk thermodynamic criteria to European Centre for Medium-Range Weather Forecasts (ECMWF) operational analyses, we provide the first global hourly climatology of potential dust devil and dusty plume (PDDP) occurrence. In agreement with observations, activity is highest from late morning into the afternoon. Combining PDDP frequencies with dust source maps and typical emission values gives the best estimate of global contributions of 3.4% (uncertainty 0.9–31%), 1 order of magnitude lower than the only estimate previously published. Total global hours of dust uplift by dry convection are ∼0.002% of the dust-lifting winds resolved by ECMWF, consistent with dry convection making a small contribution to global uplift. Reducing uncertainty requires better knowledge of factors controlling PDDP occurrence, source regions, and dust fluxes induced by dry convection. Key Points Global potential dust devil occurrence quantified from meteorological analyses Climatology shows realistic diurnal cycle and geographical distribution Best estimate of global contribution of 3.4% is 10 times smaller than the previous estimate PMID:26681815

You Can Run, But You Can't Hide Juniper Pollen Phenology and Dispersal

NASA Technical Reports Server (NTRS)

Luvall, Jeffrey C.

2013-01-01

Pollen can be transported great distances. Van de Water et. al., 2003 reported Juniperus spp. pollen was transported 200-600 km. Hence local observations of plant phenology may not be consistent with the timing and source of pollen collected by pollen sampling instruments. The DREAM (Dust REgional Atmospheric Model, Nickovic et al. 2001) is a verified model for atmospheric dust transport modeling using MODIS data products to identify source regions and quantities of dust. We are modified the DREAM model to incorporate pollen transport. Pollen release is estimated based on MODIS derived phenology of Juniperus spp. communities. Ground based observational records of pollen release timing and quantities are used as verification. This information will be used to support the Centers for Disease Control and Prevention's National Environmental Public Health Tracking Program and the State of New Mexico environmental public health decision support for asthma and allergies alerts.

Epifluorescent direct counts of bacteria and viruses from topsoil of various desert dust storm regions

USGS Publications Warehouse

Gonzalez-Martin, Cristina; Teigell-Perez, Nuria; Lyles, Mark; Valladares, Basilio; Griffin, Dale W.

2013-01-01

Topsoil from arid regions is the main source of dust clouds that move through the earth's atmosphere, and microbial communities within these soils can survive long-range dispersion. Microbial abundance and chemical composition were analyzed in topsoil from various desert regions. Statistical analyses showed that microbial direct counts were strongly positively correlated with calcium concentrations and negatively correlated with silicon concentrations. While variance between deserts was expected, it was interesting to note differences between sample sites within a given desert region, illustrating the 'patchy' nature of microbial communities in desert environments.

Iron Mineralogy and Speciation in Clay-Sized Fractions of Chinese Desert Sediments

NASA Astrophysics Data System (ADS)

Lu, Wanyi; Zhao, Wancang; Balsam, William; Lu, Huayu; Liu, Pan; Lu, Zunli; Ji, Junfeng

2017-12-01

Iron released from Asian desert dust may be an important source of bioavailable iron for the North Pacific Ocean and thereby may stimulate primary productivity. However, the Fe species of the fine dusts from this source region are poorly characterized. Here we investigate iron species and mineralogy in the clay-sized fractions (<2 μm), the size fraction most prone to long-distance transport as dust. Samples were analyzed by sequential chemical extraction, X-ray diffraction, and diffuse reflectance spectrometry. Our results show that Fe dissolved from easily reducible iron phases (ferrihydrite and lepidocrocite) and reducible iron oxides (dominated by goethite) are 0.81 wt % and 2.39 wt %, respectively, and Fe dissolved from phyllosilicates extracted by boiling HCl (dominated by chlorite) is 3.15 wt %. Dusts originating from deserts in northwestern China, particularly the Taklimakan desert, are relatively enriched in easily reducible Fe phases, probably due to abundant Fe contained in fresh weathering products resulting from the rapid erosion associated with active uplift of mountains to the west. Data about Fe speciation and mineralogy in Asian dust sources will be useful for improving the quantification of soluble Fe supplied to the oceans, especially in dust models.

Molecular gas associated with IRAS 10361-5830

NASA Astrophysics Data System (ADS)

Vazzano, M. M.; Cappa, C. E.; Vasquez, J.; Rubio, M.; Romero, G. A.

2014-10-01

Aims: We analyze the distribution of the molecular gas and dust in the molecular clump linked to IRAS 10361-5830, located in the environs of the bubble-shaped Hii region Gum 31 in the Carina region, with the aim of determining the main parameters of the associated material and of investigating the evolutionary state of the young stellar objects identified there. Methods: Using the APEX telescope, we mapped the molecular emission in the J = 3-2 transition of three CO isotopologues, 12CO, 13CO and C18O, over a 1.´5 × 1.´5 region around the IRAS position. We also observed the high-density tracers CS and HCO+ toward the source. The cold- dust distribution was analyzed using submillimeter continuum data at 870 μm obtained with the APEX telescope. Complementary IR and radio data at different wavelengths were used to complete the study of the interstellar medium. Results: The molecular gas distribution reveals a cavity and a shell-like structure of ~0.32 pc in radius centered at the position of the IRAS source, with some young stellar objects projected onto the cavity. The total molecular mass in the shell and the mean H2volume density are ~40 M⊙ and ~(1-2) × 103 cm-3. The cold-dust counterpart of the molecular shell has been detected in the far-IR at 870 μm and in Herschel data at 350 μm. Weak extended emission at 24 μm from warm dust is projected onto the cavity, as well as weak radio continuum emission. Conclusions: A comparison of the distribution of cold and warm dust, and molecular and ionized gas allows us to conclude that a compact Hii region has developed in the molecular clump, indicating that this is an area of recent massive star formation. Probable exciting sources capable of creating the compact Hii region are investigated. The 2MASS source 10380461-5846233 (MSX G286.3773-00.2563) seems to be responsible for the formation of the Hii region. FITS files with datacubes corresponding to 12CO, 13CO, C180 maps are only available at the CDS via anonymous ftp to http://cdsarc.u-strasbg.fr (ftp://130.79.128.5) or via http://cdsarc.u-strasbg.fr/viz-bin/qcat?J/A+A/570/A109

Source apportionment of fine particles and its chemical components over the Yangtze River Delta, China during a heavy haze pollution episode

NASA Astrophysics Data System (ADS)

Li, L.; An, J. Y.; Zhou, M.; Yan, R. S.; Huang, C.; Lu, Q.; Lin, L.; Wang, Y. J.; Tao, S. K.; Qiao, L. P.; Zhu, S. H.; Chen, C. H.

2015-12-01

An extremely high PM2.5 pollution episode occurred over the eastern China in January 2013. In this paper, the particulate matter source apportionment technology (PSAT) method coupled within the Comprehensive air quality model with extensions (CAMx) is applied to study the source contributions to PM2.5 and its major components at six receptors (Urban Shanghai, Chongming, Dianshan Lake, Urban Suzhou, Hangzhou and Zhoushan) in the Yangtze River Delta (YRD) region. Contributions from 4 source areas (including Shanghai, South Jiangsu, North Zhejiang and Super-region) and 9 emission sectors (including power plants, industrial boilers and kilns, industrial processing, mobile source, residential, volatile emissions, dust, agriculture and biogenic emissions) to PM2.5 and its major components (sulfate, nitrate, ammonia, organic carbon and elemental carbon) at the six receptors in the YRD region are quantified. Results show that accumulation of local pollution was the largest contributor during this air pollution episode in urban Shanghai (55%) and Suzhou (46%), followed by long-range transport (37% contribution to Shanghai and 44% to Suzhou). Super-regional emissions play an important role in PM2.5 formation at Hangzhou (48%) and Zhoushan site (68%). Among the emission sectors contributing to the high pollution episode, the major source categories include industrial processing (with contributions ranging between 12.7 and 38.7% at different receptors), combustion source (21.7-37.3%), mobile source (7.5-17.7%) and fugitive dust (8.4-27.3%). Agricultural contribution is also very significant at Zhoushan site (24.5%). In terms of the PM2.5 major components, it is found that industrial boilers and kilns are the major source contributor to sulfate and nitrate. Volatile emission source and agriculture are the major contributors to ammonia; transport is the largest contributor to elemental carbon. Industrial processing, volatile emissions and mobile source are the most significant contributors to organic carbon. Results show that the Yangtze River Delta region should focus on the joint pollution control of industrial processing, combustion emissions, mobile source emissions, and fugitive dust. Regional transport of air pollution among the cities are prominent, and the implementation of regional joint prevention and control of air pollution will help to alleviate fine particulate matter concentrations under heavy pollution case significantly.

Characterization of dustfall in rural and urban sites during three dust storms in northern China, 2010

NASA Astrophysics Data System (ADS)

Lyu, Yanli; Qu, Zhiqiang; Liu, Lianyou; Guo, Lanlan; Yang, Yanyan; Hu, Xia; Xiong, Yiying; Zhang, Guoming; Zhao, Mengdi; Liang, Bo; Dai, Jiadong; Zuo, Xiyang; Jia, Qingpan; Zheng, Hao; Han, Xujiao; Zhao, Shoudong; Liu, Qi

2017-10-01

Dust transport and deposition processes are important for understanding the environmental risk of dust storms. This study investigated characteristics of dustfall at two rural sites and four urban sites from dust sources to downwind regions during three dust storms (DS1: March 19-22, DS2: April 24-26, DS3: May 7-10, 2010). Analysis of near-surface instantaneous maximum wind speed and prevailing wind direction revealed the dust storms bursted out from northwestern arid and semiarid regions to eastern China. Microaggregates, angular, subangular, columnar, subrounded, and spherical particles were identified by scanning electron microscope. Dust deposition flux (DDF) during the dust storms was significantly high at sites near sand deserts and sandy land. During DS2, DDF was 25.1, 9.9, 2.3, and 1.5 g m-2 in Jingbian, Shapotou, Lanzhou, and Beijing, respectively. The three dust storms contributed 7.3% of Beijing's annual dustfall in 2010, which suggests anthropogenic dust might contribute the majority of annual dustfall in urban areas. The mass medium diameter of dustfall during DS2 in Shapotou, Jingbian, Lanzhou, and Beijing was 26.1, 9.0, 16.4, and 15.5 μm, respectively. Urban dustfall contained more heavy metals, sulfur and arsenic than rural dustfall. Cadmium contamination was identified in all urban dust particles. Anthropogenic pollutants in combination with mineral dust might lead to complex environmental risk on local, regional, and global scales. China's environmental pollution control should integrate reductions in land desertification and multisource anthropogenic emissions within the context of climate change mitigation.

Use of MODIS Satellite Data to Evaluate Juniperus spp. Pollen Phenology to Support a Pollen Dispersal Model, PREAM, to Support Public Health Allergy Alerts

NASA Technical Reports Server (NTRS)

Luvall, J. C.; Sprigg, W.; Levetin, E.; Huete, A.; Nickovic, S.; Pejanovic, G. A.; Vukovic, A.; VandeWater, P.; Budge, A.; Hudspeth, W.;

Quantification of Asian Dust Plume Seasonal Dynamics and Regional Features

NASA Technical Reports Server (NTRS)

Goetz, Michael

2011-01-01

Dust is but one of many aerosols that are analyzed at the Jet Propulsion Laboratory in Pasadena. The purpose of this paper is to describe the process in analyzing and digitizing dust within a source region to better explain the work achieved by my internship. This paper will go over how to view collected data by Multi-angle Imaging SpectroRadiometer (MISR) [1] and the procedure of downloading data to be analyzed. With this data, one can digitize dust plumes using two methods called plume lines and plume polygons with the help of the software MISR INteractive eXplorer (MINX)[3]; thus, the theory of MINX's[3] algorithm and these methods are discussed in detail. Research was gathered from these techniques and emphasis is also focused on the obtained data and results.

Regional prediction of carbon isotopes in soil carbonates for Asian dust source tracer

NASA Astrophysics Data System (ADS)

Chen, Bing; Cui, Xinjuan; Wang, Yaqiang

2016-10-01

Dust particles emitted from deserts and semi-arid lands in northern China cause particulate pollution that increases the burden of disease particularly for urban population in East Asia. The stable carbon isotopes (δ13C) of carbonates in soils and dust aerosols in northern China were investigated. We found that the δ13C of carbonates in surface soils in northern China showed clearly the negative correlation (R2 = 0.73) with Normalized Difference Vegetation Index (NDVI). Using Moderate Resolution Imaging Spectroradiometer (MODIS) satellite-derived NDVI, we predicted the regional distribution of δ13C of soil carbonates in deserts, sandy lands, and steppe areas. The predictions show the mean δ13C of -0.4 ± 0.7‰ in soil carbonates in Taklimakan Desert and Gobi Deserts, and the isotope values decrease to -3.3 ± 1.1‰ in sandy lands. The increase in vegetation coverage depletes 13C in soil carbonates, thus the steppe areas are predicted by the lowest δ13C levels (-8.1 ± 1.7‰). The measurements of atmospheric dust samples at eight sites showed that the Asian dust sources were well assigned by the 13C mapping in surface soils. Predicting 13C in large geographical areas with fine resolution offers a cost-effective tracer to monitor dust emissions from sandy lands and steppe areas which show an increasing role in Asian dust loading driven by climate change and human activities.

Modeling of mineral dust in the atmosphere: Sources, transport, and optical thickness

NASA Technical Reports Server (NTRS)

Tegen, Ina; Fung, Inez

1994-01-01

A global three-dimensional model of the atmospheric mineral dust cycle is developed for the study of its impact on the radiative balance of the atmosphere. The model includes four size classes of minearl dust, whose source distributions are based on the distributions of vegetation, soil texture and soil moisture. Uplift and deposition are parameterized using analyzed winds and rainfall statistics that resolve high-frequency events. Dust transport in the atmosphere is simulated with the tracer transport model of the Goddard Institute for Space Studies. The simulated seasonal variations of dust concentrations show general reasonable agreement with the observed distributions, as do the size distributions at several observing sites. The discrepancies between the simulated and the observed dust concentrations point to regions of significant land surface modification. Monthly distribution of aerosol optical depths are calculated from the distribution of dust particle sizes. The maximum optical depth due to dust is 0.4-0.5 in the seasonal mean. The main uncertainties, about a factor of 3-5, in calculating optical thicknesses arise from the crude resolution of soil particle sizes, from insufficient constraint by the total dust loading in the atmosphere, and from our ignorance about adhesion, agglomeration, uplift, and size distributions of fine dust particles (less than 1 micrometer).

Northern hemisphere dust storms on Mars

NASA Technical Reports Server (NTRS)

James, P. B.

1993-01-01

Dust storms in the northern hemisphere of Mars appear to be less common than the more familiar southern hemisphere storms, and essentially, no activity north of about 30 latittude has been documented. The data are, however, subject to an observational bias because Mars is near aphelion during oppositions, which occur during the most likely seasons for dust activity in the north. The amount of dust activity in the northern hemisphere is clearly very relevant to the role of atmospheric transport in the dust cycle. The classic global storms that occur during spring in the southern hemisphere are observed to transport dust from sources in the southern hemisphere to sinks or temporary depositories in the north. The question of whether atmospheric transport can close the dust cycle, i.e., return the dust to the southern hemisphere sources on some timescale, is clearly relevant to the solution of the puzzle of how the dust storm cycle is modulated, i.e., why storms occur in some years but not in others. There are data that suggest that the spring/early summer season in the northern hemisphere of Mars during the year following the major 1977 storms observed by Viking was very dusty. A number of observations of the vicinity of the receding north polar cap showed clear evidence of substantial dust activity in the sub-Arctic region.

Mars Dust and LETKF Data Assimilation of TES Observations

NASA Astrophysics Data System (ADS)

Greybush, S. J.; Hoffman, R. N.; Wilson, R.; Kang, J.; Zhao, Y.; Hoffman, M. J.; Kalnay, E.; Miyoshi, T.

2012-12-01

Simulation and prediction of dust storms remains one of the greatest challenges in Martian meteorology. Large-scale dust storms impact all Mars operations including spacecraft observations. What makes the difference between a regional event and a planet-encircling event? What are the predictability characteristics of these events and of the transition from regional to global? We examine the meteorology, including dustiness, in the Mars reanalysis created with the GFDL Mars Global Climate Model (MGCM) Local Ensemble Transform Kalman Filter (LETKF) data assimilation system (DAS). Characterizing the distribution and temporal evolution of dust in the Martian atmosphere is a considerable challenge. Spacecraft observations are sparse and have limitations in vertical coverage, dust physical properties are not well known, and model parameterizations of surface lifting have limited success in reproducing observed variability. Methods for generating a dust reanalysis begin with satellite inferred dust information in the form of column opacities, dust profile retrievals, or the original radiances. Opacities may be estimated from a formal retrieval of the satellite data or inferred through surface brightness temperatures. The opacities have been ingested via ad hoc adjustments to model tracer fields (Conrath vertical distributions, changes to the boundary layer dust only, etc.), but could also be assimilated by the LETKF or other advanced DAS. We will present dust distributions in the most recent version of the MGCM-LETKF Mars reanalysis. Current results are from two DASs, one assuming a fixed dust distribution and one using TES opacities and updating the boundary layer dust only. In these reanalyses, a full year of Thermal Emission Spectrometer (TES) temperature profiles have been assimilated. Since an accurate characterization of the sources and sinks of dust would greatly improve our understanding of the Martian dust cycle and its representation in numerical weather prediction models, we will examine two advanced DAS techniques that have been demonstrated in terrestrial DASs and could be applied to the problem -- surface dust flux estimation and estimating the surface parameters that control the source of dust (roughness, inventories). The surface dust flux method requires no a priori information about the fluxes, and uses only atmospheric observations. For the terrestrial CO2 problem, surface sources and sinks of CO2 have been estimated using only time-dependent measurements of atmospheric CO2, temperatures, and winds, and without a priori information on the surface fluxes. This scenario is very analogous to the case of Mars. On Mars we have only information on temperature and dust opacities at spacecraft overpass locations. Results for terrestrial CO2 and plans for Mars dust will be presented. However, to improve model parameterizations of dust lifting, we need to understand not only the planetary distribution of dust but also the evolution of its sources and sinks and their relation to meteorology. The surface parameters method assumes the physical properties have a persistence or damped persistence evolution equation. These are then treated as part of the model state vector in the LETKF. This approach is then analogous to the bias correction method used in LETKF to improve the atmospheric state estimation.

Simulating Dust Regional Impact on the Middle East Climate and the Red Sea

NASA Astrophysics Data System (ADS)

Osipov, Sergey; Stenchikov, Georgiy

2017-04-01

Dust is one of the most abundant aerosols, however, currently only a few regional climate downscalings account for dust. This study focuses on the Middle East and the Red Sea regional climate response to the dust aerosol radiative forcing. The Red Sea is located between North Africa and Arabian Peninsula, which are first and third largest source regions of dust, respectively. MODIS and SEVIRI satellite observations show extremely high dust optical depths in the region, especially over the southern Red Sea during the summer season. The significant north-to-south gradient of the dust optical depth over the Red Sea persists throughout the entire year. Modeled atmospheric radiative forcing at the surface, top of the atmosphere and absorption in the atmospheric column indicate that dust significantly perturbs radiative balance. Top of the atmosphere modeled forcing is validated against independently derived GERB satellite product. Due to strong radiative forcing at the sea surface (daily mean forcing during summer reaches -32 Wm-2 and 10 Wm-2 in SW and LW, respectively), using uncoupled ocean model with prescribed atmospheric boundary conditions would result in an unrealistic ocean response. Therefore, here we employ the Regional Ocean Modeling system (ROMS) fully coupled with the Weather Research and Forecasting (WRF) model to study the impact of dust on the Red Sea thermal regime and circulation. The WRF was modified to interactively account for the radiative effect of dust. Daily spectral optical properties of dust are computed using Mie, T-matrix, and geometric optics approaches, and are based on the SEVIRI climatological optical depth. The WRF model parent and nested domains are configured over the Middle East and North Africa (MENA) region and over the Red Sea with 30 and 10 km resolution, respectively. The ROMS model over the Red Sea has 2 km grid spacing. The simulations show that, in the equilibrium response, dust causes 0.3-0.5 K cooling of the Red Sea surface waters, and weakens the overturning circulation in the Red Sea. The salinity distribution, freshwater, and heat budgets are significantly perturbed. This indicates that dust plays an important role in the formation of the Red Sea energy balance and circulation regimes, and has to be thoroughly accounted for in future modeling studies.

Impacts of Dust on Tropical Volcanic Soil Formation: Insights from Strontium and Uranium-Series Isotopes in Soils from Basse-Terre Island, French Guadeloupe

NASA Astrophysics Data System (ADS)

Pereyra, Y.; Ma, L.; Sak, P. B.; Gaillardet, J.; Buss, H. L.; Brantley, S. L.

2015-12-01

Dust inputs play an important role in soil formation, especially for thick soils developed on tropical volcanic islands. In these regions, soils are highly depleted due to intensive chemical weathering, and mineral nutrients from dusts have been known to be important in sustaining soil fertility and productivity. Tropical volcanic soils are an ideal system to study the impacts of dust inputs on the ecosystem. Sr and U-series isotopes are excellent tracers to identify sources of materials in an open system if the end-members have distinctive isotope signatures. These two isotope systems are particularly useful to trace the origin of atmospheric inputs into soils and to determine rates and timescales of soil formation. This study analyzes major elemental concentrations, Sr and U-series isotope ratios in highly depleted soils in the tropical volcanic island of Basse-Terre in French Guadeloupe to determine atmospheric input sources and identify key soil formation processes. We focus on three soil profiles (8 to 12 m thick) from the Bras-David, Moustique Petit-Bourg, and Deshaies watersheds; and on the adjacent rivers to these sites. Results have shown a significant depletion of U, Sr, and major elements in the deep profile (12 to 4 m) attributed to rapid chemical weathering. The top soil profiles (4 m to the surface) all show addition of elements such as Ca, Mg, U, and Sr due to atmospheric dust. More importantly, the topsoil profiles have distinct Sr and U-series isotope compositions from the deep soils. Sr and U-series isotope ratios of the top soils and sequential extraction fractions confirm that the sources of the dust are from the Saharan dessert, through long distance transport from Africa to the Caribbean region across the Atlantic Ocean. During the transport, some dust isotope signatures may also have been modified by local volcanic ashes and marine aerosols. Our study highlights that dusts and marine aerosols play important roles in element cycles and nutrient sources in the highly depleted surface soils of tropical oceanic islands.

The deep space 1 encounter with comet 19P/Borrelly

USGS Publications Warehouse

Boice, D.C.; Soderblom, L.A.; Britt, D.T.; Brown, R.H.; Sandel, B.R.; Yelle, R.V.; Buratti, B.J.; Hicks, M.D.; Nelson, R.M.; Rayman, M.D.; Oberst, J.; Thomas, N.

2002-01-01

NASA's Deep Space 1 (DS1) spacecraft successfully encountered comet 19P/Borrelly near perihelion and the Miniature Integrated Camera and Spectrometer (MICAS) imaging system onboard DS1 returned the first high-resolution images of a Jupiter-family comet nucleus and surrounding environment. The images span solar phase angles from 88?? to 52??, providing stereoscopic coverage of the dust coma and nucleus. Numerous surface features are revealed on the 8-km long nucleus in the highest resolution images (47-58 m/pixel). A smooth, broad basin containing brighter regions and mesa-like structures is present in the central part of the nucleus that seems to be the source of jet-like dust features seen in the coma. High ridges seen along the jagged terminator lead to rugged terrain on both ends of the nucleus containing dark patches and smaller series of parallel grooves. No evidence of impact craters with diameters larger than about 200-m are present, indicating a young and active surface. The nucleus is very dark with albedo variations from 0.007 to 0.035. Short-wavelength, infrared spectra from 1.3 to 2.6 ??m revealed a hot, dry surface consistent with less than about 10% actively sublimating. Two types of dust features are seen: Broad fans and highly collimated "jets" in the sunward hemisphere that can be traced to the surface. The source region of the main jet feature, which resolved into at least three smaller "jets" near the surface, is consistent with an area around the rotation pole that is constantly illuminated by the sun during the encounter. Within a few nuclear radii, entrained dust is rapidly accelerated and fragmented and geometrical effects caused from extended source regions are present, as evidenced in radial intensity profiles centered on the jet features that show an increase in source strength with increasing cometocentric distance. Asymmetries in the dust from dayside to nightside are pronounced and may show evidence of lateral flow transporting dust to structures observed in the nightside coma. A summary of the initial results of the Deep Space 1 Mission is provided, highlighting the new knowledge that has been gained thus far.

Uncertainty in Modeling Dust Mass Balance and Radiative Forcing from Size Parameterization

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zhao, Chun; Chen, Siyu; Leung, Lai-Yung R.

2013-11-05

This study examines the uncertainties in simulating mass balance and radiative forcing of mineral dust due to biases in the aerosol size parameterization. Simulations are conducted quasi-globally (180oW-180oE and 60oS-70oN) using the WRF24 Chem model with three different approaches to represent aerosol size distribution (8-bin, 4-bin, and 3-mode). The biases in the 3-mode or 4-bin approaches against a relatively more accurate 8-bin approach in simulating dust mass balance and radiative forcing are identified. Compared to the 8-bin approach, the 4-bin approach simulates similar but coarser size distributions of dust particles in the atmosphere, while the 3-mode pproach retains more finemore » dust particles but fewer coarse dust particles due to its prescribed og of each mode. Although the 3-mode approach yields up to 10 days longer dust mass lifetime over the remote oceanic regions than the 8-bin approach, the three size approaches produce similar dust mass lifetime (3.2 days to 3.5 days) on quasi-global average, reflecting that the global dust mass lifetime is mainly determined by the dust mass lifetime near the dust source regions. With the same global dust emission (~6000 Tg yr-1), the 8-bin approach produces a dust mass loading of 39 Tg, while the 4-bin and 3-mode approaches produce 3% (40.2 Tg) and 25% (49.1 Tg) higher dust mass loading, respectively. The difference in dust mass loading between the 8-bin approach and the 4-bin or 3-mode approaches has large spatial variations, with generally smaller relative difference (<10%) near the surface over the dust source regions. The three size approaches also result in significantly different dry and wet deposition fluxes and number concentrations of dust. The difference in dust aerosol optical depth (AOD) (a factor of 3) among the three size approaches is much larger than their difference (25%) in dust mass loading. Compared to the 8-bin approach, the 4-bin approach yields stronger dust absorptivity, while the 3-mode approach yields weaker dust absorptivity. Overall, on quasi-global average, the three size parameterizations result in a significant difference of a factor of 2~3 in dust surface cooling (-1.02~-2.87 W m-2) and atmospheric warming (0.39~0.96 W m-2) and in a tremendous difference of a factor of ~10 in dust TOA cooling (-0.24~-2.20 W m-2). An uncertainty of a factor of 2 is quantified in dust emission estimation due to the different size parameterizations. This study also highlights the uncertainties in modeling dust mass and number loading, deposition fluxes, and radiative forcing resulting from different size parameterizations, and motivates further investigation of the impact of size parameterizations on modeling dust impacts on air quality, climate, and ecosystem.« less

An ALMA Survey of Protoplanetary Disks in the σ Orionis Cluster

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ansdell, M.; Williams, J. P.; Marel, N. van der

2017-05-01

The σ  Orionis cluster is important for studying protoplanetary disk evolution, as its intermediate age (∼3–5 Myr) is comparable to the median disk lifetime. We use ALMA to conduct a high-sensitivity survey of dust and gas in 92 protoplanetary disks around σ  Orionis members with M {sub *} ≳ 0.1  M {sub ⊙}. Our observations cover the 1.33 mm continuum and several CO J  = 2–1 lines: out of 92 sources, we detect 37 in the millimeter continuum and 6 in {sup 12}CO, 3 in {sup 13}CO, and none in C{sup 18}O. Using the continuum emission to estimate dust mass, we find only 11more » disks with M {sub dust} ≳ 10  M {sub ⊕}, indicating that after only a few Myr of evolution most disks lack sufficient dust to form giant planet cores. Stacking the individually undetected continuum sources limits their average dust mass to 5×  lower than that of the faintest detected disk, supporting theoretical models that indicate rapid dissipation once disk clearing begins. Comparing the protoplanetary disk population in σ  Orionis to those of other star-forming regions supports the steady decline in average dust mass and the steepening of the M {sub dust}– M {sub *} relation with age; studying these evolutionary trends can inform the relative importance of different disk processes during key eras of planet formation. External photoevaporation from the central O9 star is influencing disk evolution throughout the region: dust masses clearly decline with decreasing separation from the photoionizing source, and the handful of CO detections exist at projected separations of >1.5 pc. Collectively, our findings indicate that giant planet formation is inherently rare and/or well underway by a few Myr of age.« less

Subjective Mapping of Dust-Emission Sources by Using MODIS Imagery

DTIC Science & Technology

2017-05-01

within the inset of Panel A. Panel A is a True Color image that depicts white clouds against a brown landscape; a bird’s eye representation of Earth...shows the location of the Hamun dry lakes, which are an important dust source in the region. The enlarged image box in the top right depicts the...Bacon and McDonald 2016). For example, dry lakebeds filled with unconsolidated ERDC/CRREL TR-17-8 4 fine-grained sediments are commonly

Hot Dust in Ultraluminous Infrared Galaxies

NASA Astrophysics Data System (ADS)

Shchekinov, Yu. A.; Vasiliev, E. O.

2017-12-01

Ultraluminous infrared galaxies with total luminosities an order of magnitude greater than that of our galaxy over wavelengths of λλ = 10-800 μm are characterized by a high mass concentration of dust. Because of this, the optical thickness of the interstellar gas is extremely high, especially in the central regions of the galaxies, ranging from 1 at millimeter wavelengths to 104 in the visible. The average temperature of the dust in them is about Td=30 K, but the variations from one galaxy to another are large, with Td=20-70 K. The main source of dust in these galaxies seems to be type II supernova bursts and the main heating source is stars. In addition, given that shock waves from supernovae are an effective mechanism for destruction of interstellar dust in our galaxy and the high optical thickness of the gas with respect to the heating radiation from the stars, this conclusion merits detailed analysis. This paper provides estimates of the dust mass balance and details of its heating in these galaxies based on the example of the ultraluminous galaxy closest to us, Arp 220. It is shown that when supernovae are dominant in the production and destruction of dust in the interstellar gas, the resultant dust mass fraction is close to the observed value for Arp 220. It is also found that the observed stellar population of this galaxy can support a high ( Td ≃ 67 K ) temperature if the dust in its central region is concentrated in small, dense (n 105 cm-3) clouds with radii of 0.003 ≲ pc. Mechanisms capable of maintaining an interstellar gas structure in this state are discussed.

Investigating the 'Iron Hypothesis' in the North Pacific: Trans-Pacific Dust and Methanesulfonate (MSA) in the Denali Ice Core, Alaska

NASA Astrophysics Data System (ADS)

Saylor, P. L.; Osterberg, E. C.; Winski, D.; Ferris, D. G.; Koffman, B. G.; Kreutz, K. J.; Wake, C. P.; Campbell, S. W.

2015-12-01

Oceanic deposition of Asian-sourced, Iron-rich dust particulate has been linked to enhanced phytoplankton productivity in regions of the Pacific Ocean. High Nutrient Low Chlorophyll (HNLC) ocean regions, such as the North Pacific, are hypothesized to play a significant role in changing atmospheric CO­2 concentrations on glacial-interglacial timescales. Phytoplankton blooms generate methanesulfonate (MSA), an atmospheric oxidation product of dimethylsulfide (DMS) that is readily aerosolized and deposited in nearby glacial ice. In the summer of 2013, an NSF-funded team from Dartmouth College and the Universities of Maine and New Hampshire collected two 1000 year-long parallel ice cores to bedrock from the summit plateau of Mount Hunter in Denali National Park, Alaska (62.940° N, 151.088° W, 3912 m elevation). The Mt. Hunter ice core site is well situated to record changes in trans-Pacific dust flux and MSA emissions in the North Pacific. Here we investigate the history of dust flux to Denali over the last millennium using major and trace element chemistry and microparticle concentration and size distribution data from the Mt. Hunter cores. We evaluate potential controlling mechanisms on Denali dust flux including conditions at Asian dust sources (storminess, wind speed, precipitation), the strength of the Aleutian Low, and large-scale climate modes such as the El Niño-Southern Oscillation and the Pacific Decadal Oscillation. We also evaluate the Mt. Hunter record for relationships between dust flux and MSA concentrations to investigate whether dust fertilization enhanced North Pacific phytoplankton production over the past 1000 years. Future work will create a composite North Pacific dust record using new and existing Mt. Logan ice core records to evaluate these relationships over the entire Holocene.

A mini outburst from the nightside of comet 67P/Churyumov-Gerasimenko observed by the OSIRIS camera on Rosetta

NASA Astrophysics Data System (ADS)

Knollenberg, J.; Lin, Z. Y.; Hviid, S. F.; Oklay, N.; Vincent, J.-B.; Bodewits, D.; Mottola, S.; Pajola, M.; Sierks, H.; Barbieri, C.; Lamy, P.; Rodrigo, R.; Koschny, D.; Rickman, H.; A'Hearn, M. F.; Barucci, M. A.; Bertaux, J. L.; Bertini, I.; Cremonese, G.; Davidsson, B.; Da Deppo, V.; Debei, S.; De Cecco, M.; Fornasier, S.; Fulle, M.; Groussin, O.; Gutiérrez, P. J.; Ip, W.-H.; Jorda, L.; Keller, H. U.; Kührt, E.; Kramm, J. R.; Küppers, M.; Lara, L. M.; Lazzarin, M.; Lopez Moreno, J. J.; Marzari, F.; Naletto, G.; Thomas, N.; Güttler, C.; Preusker, F.; Scholten, F.; Tubiana, C.

2016-12-01

Context. On 12 March 2015 the OSIRIS WAC camera onboard the ESA Rosetta spacecraft orbiting comet 67P/Churyumov-Gerasimenko observed a small outburst originating from the Imhotep region at the foot of the big lobe of the comet. These measurements are unique since it was the first time that the initial phase of a transient outburst event could be directly observed. Aims: We investigate the evolution of the dust jet in order to derive clues about the outburst source mechanism and the ejected dust particles, in particular the dust mass, dust-to-gas ratio and the particle size distribution. Methods: Analysis of the images and of the observation geometry using comet shape models in combination with gasdynamic modeling of the transient dust jet were the main tools used in this study. Synthetic images were computed for comparison with the observations. Results: Analysis of the geometry revealed that the source region was not illuminated until 1.5 h after the event implying true nightside activity was observed. The outburst lasted for less than one hour and the average dust production rate during the initial four minutes was of the order of 1 kg/s. During this time the outburst dust production rate was approximately constant, no sign for an initial explosion could be detected. For dust grains between 0.01-1 mm a power law size distribution characterized by an index of about 2.6 provides the best fit to the observed radiance profiles. The dust-to-gas ratio of the outburst jet is in the range 0.6-1.8.

Variations on morphology and elemental composition of mineral dust particles from local, regional, and long-range transport meteorological scenarios

NASA Astrophysics Data System (ADS)

Coz, Esther; Gómez-Moreno, Francisco J.; Casuccio, Gary S.; ArtíñAno, BegoñA.

2010-06-01

Mineral dust is the second major source of PM10 in Madrid, reaching up to 80% of the PM10 mass during certain long-range dust transport events. Three different types of scenarios have been found to be associated with the high particle concentration episodes in the city: local anthropogenic, regional recirculation, and African dust transport processes. The present study focuses on the characterization of the individual mineral dust particles related to some chemical and morphological features during these three types of episodes, with special attention to local and regional episodes. To achieve this purpose, four different samples were selectively collected during the 2004-2005 period campaigns, one corresponding to each type of scenario and other sample from an Atlantic ventilated one. Meteorological situation, dust source identification, impact on ambient concentrations, size range distribution, and particle individual analysis have been characterized for each of them. Elemental composition and morphology of more than 30,000 mineral particles were analyzed by computer-controlled scanning electron microscopy. Particles were grouped into clusters based on their elemental composition, and the aspect ratio (AR) of each cluster or category was compared for each type of episode. The AR was related to the mineralogical crystal structure of each chemical cluster. The dates chosen for microscopy analysis were in good agreement in size distribution and chemical composition with the average of the dates in the entire campaign and with those from previous campaigns. Major differences between local/regional and long-range transported mineral dust were found in the relative abundance between carbonates and silicates, with much higher abundance of calcium carbonates in the first ones. These differences between silicate and carbonate contents were consistent with the results found in previous campaigns and were directly related to the composition of the parent topsoil by studying the Ca/Si ratios of similar episodes recorded all over the Iberian Peninsula. Differences in morphology were also found for these scenarios. The predominance of calcium carbonate under regional and local influence is scientifically relevant since this mineral is known to react with both SO2 and HNO3 in the atmosphere. Larger average AR values were found for dust particles from long-range transport, and smaller average AR values were found for particles from local and regional resuspended dust. The increasing average AR value has been linked to the silicate cluster presence, whereas a reduction has been observed within the carbonate cluster.

Overview of Dust Model Inter-comparison (DMIP) in East Asia

NASA Astrophysics Data System (ADS)

Uno, I.

2004-12-01

Dust transport modeling plays an important role in understanding the recent increase of Asian Dust episodes and its impact to the regional climate system. Several dust models have been developed in several research institutes and government agencies independently since 1990s. Their numerical results either look very similar or different. Those disagreements are caused by difference in dust modules (concepts and basic mechanisms) and atmospheric models (meteorological and transport models). Therefore common understanding of performance and uncertainty of dust erosion and transport models in the Asian region becomes very important. To have a better understanding of dust model application, we proposed the dust model intercomparison under the international cooperation networks as a part of activity of ADEC (Aeolian Dust Experiment on Climate Impact) project research. Current participants are Kyusyu Univ. (Japan), Meteorological Research Institute (Japan), Hong-Kong City Univ. (China), Korean Meteorological Agency METRI (Korea), US Naval Research Laboratory (USA), Chinese Meteorological Agency (China), Institute of Atmospheric Physics (China), Insular Coastal Dynamics (Malta) and Meteorological Service of Canada (Canada). As a case study episode, we set two huge dust storms occurred in March and April 2002. Results from the dust transport model from all the participants are compiled on the same methods and examined the model characteristics against the ground and airborne measurement data. We will also examine the dust model results from the horizontal distribution at specified levels, vertical profiles, concentration at special check point and emission flux at source region, and show the important parameters for dust modeling. In this paper, we will introduce the general overview of this DMIP activity and several important conclusions from this activity.

A parallel direct numerical simulation of dust particles in a turbulent flow

NASA Astrophysics Data System (ADS)

Nguyen, H. V.; Yokota, R.; Stenchikov, G.; Kocurek, G.

2012-04-01

Due to their effects on radiation transport, aerosols play an important role in the global climate. Mineral dust aerosol is a predominant natural aerosol in the desert and semi-desert regions of the Middle East and North Africa (MENA). The Arabian Peninsula is one of the three predominant source regions on the planet "exporting" dust to almost the entire world. Mineral dust aerosols make up about 50% of the tropospheric aerosol mass and therefore produces a significant impact on the Earth's climate and the atmospheric environment, especially in the MENA region that is characterized by frequent dust storms and large aerosol generation. Understanding the mechanisms of dust emission, transport and deposition is therefore essential for correctly representing dust in numerical climate prediction. In this study we present results of numerical simulations of dust particles in a turbulent flow to study the interaction between dust and the atmosphere. Homogenous and passive dust particles in the boundary layers are entrained and advected under the influence of a turbulent flow. Currently no interactions between particles are included. Turbulence is resolved through direct numerical simulation using a parallel incompressible Navier-Stokes flow solver. Model output provides information on particle trajectories, turbulent transport of dust and effects of gravity on dust motion, which will be used to compare with the wind tunnel experiments at University of Texas at Austin. Results of testing of parallel efficiency and scalability is provided. Future versions of the model will include air-particle momentum exchanges, varying particle sizes and saltation effect. The results will be used for interpreting wind tunnel and field experiments and for improvement of dust generation parameterizations in meteorological models.

Hourly elemental concentrations in PM2.5 aerosols sampled simultaneously at urban background and road site

NASA Astrophysics Data System (ADS)

Dall'Osto, M.; Querol, X.; Amato, F.; Karanasiou, A.; Lucarelli, F.; Nava, S.; Calzolai, G.; Chiari, M.

2012-08-01

Hourly-resolved aerosol chemical speciation data can be a highly powerful tool to determine the source origin of atmospheric pollutants in urban Environments. Aerosol mass concentrations of seventeen elements (Na, Mg, Al, S, Cl, K, Ca, Ti, V, Cr, Mn, Fe, Ni, Cu, Zn, Sr and Pb) were obtained by time (1 h) and size (PM2.5 particulate matter <2.5 μm) resolved Particle Induced X-ray Emission (PIXE) measurements. In the Marie Curie FP7-EU framework of SAPUSS (Solving Aerosol Problems by Using Synergistic Strategies), the unique approach used is the simultaneous PIXE measurements at two monitoring sites: urban background (UB) and a street canyon traffic road site (RS). Elements related to primary non exhaust traffic emission (Fe, Cu), dust resuspension (Ca) and anthropogenic Cl were found enhanced at the RS, whereas industrial related trace metals (Zn, Pb, Mn) were found at higher concentrations at the more ventilated UB site. When receptor modelling was performed with positive matrix factorization (PMF), nine different aerosol sources were identified at both sites: three types of regional aerosols (secondary sulphate (S) - 27%, biomass burning (K) - 5%, sea salt (Na-Mg) - 17%), three types of dust aerosols (soil dust (Al-Ti) - 17%, urban crustal dust (Ca) - 6%, and primary traffic non exhaust brake dust (Fe-Cu) - 7%), and three types industrial aerosol plumes-like events (shipping oil combustion (V-Ni) - 17%, industrial smelters (Zn-Mn) - 3%, and industrial combustion (Pb-Cl) - 5%). The validity of the PMF solution of the PIXE data is supported by strong correlations with external single particle mass spectrometry measurements. Beside apportioning the aerosol sources, some important air quality related conclusions can be drawn about the PM2.5 fraction simultaneously measured at the UB and RS sites: (1) the regional aerosol sources impact both monitoring sites at similar concentrations regardless their different ventilation conditions; (2) by contrast, local industrial aerosol plumes associated with shipping oil combustion and smelters activities have a higher impact on the more ventilated UB site; (3) a unique source of Pb-Cl (associated with industrial combustion emissions) is found a to be the major (82%) source of Cl in the urban agglomerate; (4) PM2.5 traffic brake dust (Fe-Cu) is mainly primarily emitted and not resuspended, whereas PM2.5 urban crustal dust (Ca) is found mainly resuspended by both traffic vortex and sea breeze; (5) urban dust (Ca) is found the aerosol source most affected by land wetness, reduced by a factor of eight during rainy days and suggesting that wet roads may be a solution for reducing dust concentrations in road sites, far more effective than street sweeping activities.

Iceland as the largest source of natural air pollution in the Arctic

NASA Astrophysics Data System (ADS)

Dagsson Waldhauserova, Pavla; Meinander, Outi; Olafsson, Haraldur; Arnalds, Olafur

2017-04-01

Arctic aerosols are often attributed to the Arctic Haze and long-range transport tracers. There is, however, an important dust source in the Arctic/Sub-arctic region which should receive more attention. The largest desert in the Arctic as well as in the Europe is Iceland with > 40,000 km2 of desert areas. The mean dust suspension frequency was 135 dust days annually in 1949-2012 with decreasing numbers in 2013-2015. The annual dust deposition was calculated as 31-40 million tons yr-1 affecting the area of > 500,000 km2. Satelite MODIS pictures have revealed dust plumes traveling > 1000 km at times. The physical properties of Icelandic dust showed differences in mineralogy, geochemical compositions, shapes, sizes, and colour, compared to the crustal mineral dust. Icelandic dust is of volcanic origin, dark in colour with sharp-tipped shards and large bubbles. About 80% of the particulate matter is volcanic glass rich in heavy metals, such as iron and titanium. Suspended dust measured at the glacial dust source consisted of such high number of close-to-ultrafine particles as concentrations during active eruptions. Generally, about 50% of the suspended PM10 are submicron particles in Iceland. Contrarily, suspended grains > 2 mm were captured during severe dust storm after the 2010 Eyjafjallajokull eruption when the aeolian transport exceeded 11 t m-1 of materials and placed this storms among the most extreme wind erosion events recorded on Earth. Our reflectance measurements showed that Icelandic dust deposited on snow lowers the snow albedo and reduces the snow density as much as Black Carbon. Icelandic volcanic dust tends to act as a positive climate forcing agent, both directly and indirectly, which is different to what generally concluded for crustal dust in the 2013 IPCC report. The high frequency, severity and year-round activity of volcanic dust emissions suggest that Icelandic dust may contribute to Arctic warming.

Composition and origin of PM10 in Cape Verde: Characterization of long-range transport episodes

NASA Astrophysics Data System (ADS)

Salvador, P.; Almeida, S. M.; Cardoso, J.; Almeida-Silva, M.; Nunes, T.; Cerqueira, M.; Alves, C.; Reis, M. A.; Chaves, P. C.; Artíñano, B.; Pio, C.

2016-02-01

A receptor modelling study was performed to identify source categories and their contributions to the PM10 total mass at the Cape Verde archipelago. Trajectory statistical methods were also used to characterize the main atmospheric circulation patterns causing the transport of air masses and to geographically identify the main potential source areas of each PM10 source category. Our findings point out that the variability of the PM10 levels at Cape Verde was prompted by the advections of African mineral dust. The mineral dust load was mainly composed by clay-silicates mineral derived elements (22% of the PM10 total mass on average) with lower amounts of carbonates (9%). A clear northward gradient was observed in carbonates concentration that illustrates the differences in the composition according to the source regions of mineral dust. Mineral dust was frequently linked to industrial emissions from crude oil refineries, fertilizer industries as well as oil and coal power plants, located in the northern and north-western coast of the African continent (29%). Sea salt was also registered in the PM10 mass during most part of the sampling period, with a lower impact in the PM10 levels than the mineral dust one (26%). Combustion aerosols (6%) reached the highest mean values in summer as a consequence of the emissions from local-regional sources. Biomass burning aerosols produced from October to November in sub-sahelian latitudes, had a clear influence in the content of elemental carbon (EC) recorded at Cape Verde but a small impact in the PM10 total mass levels. A minor contribution to the PM10 mass has been associated to secondary inorganic compounds-SIC. Namely, ammonium sulfate and nitrate (SIC 1-5%) and calcium sulfate and nitrate (SIC 2-3%). The main origin of SIC 1 was attributed to emissions of SO2 and NOx from industrial sources located in the northern and north-western African coast and from wildfires produced in the continent. SIC 2 had a clear regional origin in the summer period. However, in the winter period there were probably contributions of soil emissions of evaporate minerals from regions of eastern Algeria. The location of Cape Verde in the Atlantic Ocean at subtropical latitudes, and the absence of relevant local sources of anthropogenic atmospheric pollutants, becomes this archipelago, a perfect site to study the impact of external contributions on the background levels of PM10 registered over the north-eastern tropical Atlantic.

Eastern Equatorial Pacific Dust Provenance on Deglacial Timescales

NASA Astrophysics Data System (ADS)

Xie, R.; Marcantonio, F.

2008-12-01

Changing patterns of eolian dust deposition preserved in deep-sea sediments have the potential to provide us with a better understanding of changes in past atmospheric circulation. One way in which to determine the provenance of dust in deep-sea sediments is to use radiogenic isotopic tracers which can fingerprint potential dust sources. Models (e.g., [1]) suggest that sources of dust to the Eastern Equatorial Pacific (EEP) are from areas as diverse as Asia, North, Central, and South America, and, perhaps, even Africa. Here, we investigate spatial and temporal changes in the provenance of the eolian component in the EEP by measuring Pb, Sr, and Nd isotope ratios in dust extracted from sediments along a transect at 110oW from 7oN to 3oS (ODP sites 853 - 848). In this region, although fluxes of dust were higher during the last glacial maximum (LGM) than those in the Holocene by up to 100%, the glacial flux of dust displayed a shallower meridional gradient [2]. However, it is unclear whether this shallower gradient is due to a mean southerly displacement of the Intertropical Convergence Zone (ITCZ). Most of the dust trying to pass through the ITCZ will be scavenged and rained out at the ITCZ. Along the meridional gradient, therefore, temporal variations in the Pb, Sr, and Nd isotopic fingerprints of the distinct dust sources will determine the extent to which the position of the ITCZ changes on deglacial timescales. [1] Mahowald et al., 2005, Global Biogeochemical Cycles 19, GB4025. [2] McGee et al., 2007, EPSL 257, 215-230.

Concentrations and source apportionment of PM10 and associated elemental and ionic species in a lignite-burning power generation area of southern Greece.

PubMed

Argyropoulos, G; Grigoratos, Th; Voutsinas, M; Samara, C

2013-10-01

Ambient concentrations of PM10 and associated elemental and ionic species were measured over the cold and the warm months of 2010 at an urban and two rural sites located in the lignite-fired power generation area of Megalopolis in Peloponnese, southern Greece. The PM10 concentrations at the urban site (44.2 ± 33.6 μg m(-3)) were significantly higher than those at the rural sites (23.7 ± 20.4 and 22.7 ± 26.9 μg m(-3)). Source apportionment of PM10 and associated components was accomplished by an advanced computational procedure, the robotic chemical mass balance model (RCMB), using chemical profiles for a variety of local fugitive dust sources (power plant fly ash, flue gas desulfurization wet ash, feeding lignite, infertile material from the opencast mines, paved and unpaved road dusts, soil), which were resuspended and sampled through a PM10 inlet onto filters and then chemically analyzed, as well as of other common sources such as vehicular traffic, residential oil combustion, biomass burning, uncontrolled waste burning, marine aerosol, and secondary aerosol formation. Geological dusts (road/soil dust) were found to be major PM10 contributors in both the cold and warm periods of the year, with average annual contribution of 32.6 % at the urban site vs. 22.0 and 29.0 % at the rural sites. Secondary aerosol also appeared to be a significant source, contributing 22.1 % at the urban site in comparison to 30.6 and 28.7 % at the rural sites. At all sites, the contribution of biomass burning was most significant in winter (28.2 % at the urban site vs. 14.6 and 24.6 % at the rural sites), whereas vehicular exhaust contribution appeared to be important mostly in the summer (21.9 % at the urban site vs. 11.5 and 10.5 % at the rural sites). The highest contribution of fly ash (33.2 %) was found at the rural site located to the north of the power plants during wintertime, when winds are favorable. In the warm period, the highest contribution of fly ash was found at the rural site located to the south of the power plants, although it was less important (7.2 %). Moderate contributions of fly ash were found at the urban site (5.4 and 2.7 % in the cold and the warm period, respectively). Finally, the mine field was identified as a minor PM10 source, occasionally contributing with lignite dust and/or deposited wet ash dust under dry summer conditions, with the summertime contributions ranging between 3.1 and 11.0 % among the three sites. The non-parametric bootstrapped potential source contribution function analysis was further applied to localize the regions of sources apportioned by the RCMB. For the majority of sources, source regions appeared as being located within short distances from the sampling sites (within the Peloponnesse Peninsula). More distant Greek areas of the NNE sector also appeared to be source regions for traffic emissions and secondary calcium sulfate dust.

The effect of mineral dust transport on PM10 concentrations and physical properties in Istanbul during 2007-2014

NASA Astrophysics Data System (ADS)

Flores, Rosa M.; Kaya, Nefel; Eşer, Övgü; Saltan, Şehnaz

2017-11-01

Mineral dust is the most significant source of natural particulate matter. In urban regions, where > 50% of the world population is currently living, local emissions of particulate matter are further aggravated by mineral dust loadings from deserts. The megacity of Istanbul is located in an area sensitive to local pollution due to transportation (i.e., private cars, public transportation, aircrafts, ships, heavy diesel trucks, etc.), industrial emissions, residential heating, and long-range transport from Europe, Asia, and deserts. In this work, the effect of desert dust transport on PM10 concentrations and physical properties was investigated for the period of 2007-2014 in the touristic area of Aksaray, Istanbul. The Dust Regional Atmospheric Model (DREAM8b) was used to predict dust loading in Istanbul during dust transport events. Variations on surface PM10 concentrations were investigated according to seasons and during dust transport events. Cluster analysis of air mass backward trajectories was useful to understand frequency analysis and air mass trajectory dependence of PM10 concentrations on dust loadings. The effect of desert dust transport on aerosol optical depths was also investigated. It was observed that PM10 concentrations exceeded the air quality standard of 50 μg m- 3 50% of the time during the study period. The largest number of exceedances in air quality standard occurred during the spring and winter seasons. Approximately 40-60% of the dust loading occurs during the spring. Desert dust and non-desert dust sources contribute to 22-72% and 48-81% of the ground-level PM10 concentrations in Aksaray, Istanbul during the study period. Averaged AOD observed during dust transport events in spring and summer ranged 0.35-0.55. Cluster analysis resolved over 82% the variability of individual air mass backward trajectories into 5 clusters. Overall, air masses arriving to Istanbul at 500 m are equally distributed into northern (52%) and southern (48%). Frequency analysis of PM10 concentrations with mean air mass backward trajectories showed that PM10 from local anthropogenic sources may be enhanced by long-range transport from the African Desert, Asian Desert, Arabian Peninsula, Russia, and Ukraine. The work presented here provides the first integrated assessment for evaluation of occurrence and quantification of the effect of dust transport to ground-level PM10 concentrations in Istanbul, which is helpful for human health prevention and implementation of air quality control measures.

A synoptic climatology of desert dust deposition to the alpine snowpack in the San Juan Mountains, Colorado, U.S.A.

NASA Astrophysics Data System (ADS)

McBride, K.; Painter, T.; Landry, C.

2005-12-01

Currently, collaborative research is underway in the San Juan Mountains to study the radiative and hydrologic effects of desert dust deposits in alpine snow. The component described here will present preliminary results of the development of a synoptic climatology for winter and spring dust deposition to the alpine snowpack in the San Juan Mountains of southwest Colorado. An understanding of the climatology of dust deposition events will improve our capacity to infer the temporal persistence and magnitude of dust deposition and ultimately its effect on hydrologic and ecological processes in the San Juan Mountains. We use the Stochastic Time-Inverted Lagrangian Transport (STILT) model to determine back and forward trajectories of air parcels. The input data were collected at the Putney Data site (3757 m) which has been in use for over 30 years and provides 'free air' wind data as well as ridge crest air temperatures and humidity. Putney lies 2 km SE of the Swamp Angel Study Plot, east of US Highway 550 at Red Mountain Pass. The Swamp Angel Study Plot is one of two extensively instrumented energy balance and radiation sites used in the study and operated by the Center for Snow and Avalanche Studies (CSAS). STILT outputs 3-dimensional probability distributions that describe the potential source regions for air parcels reaching the San Juan Mountains at known times of dust deposition. We analyze 11 dust deposition events that have been documented in snow in the San Juan Mountains or Elk Range of Colorado. One isolated dust event was documented in 1999 in the Elk Range. Subsequently, we have documented the dust deposition events in winters and springs of 2003, 2004, and 2005 in the San Juan Mountains. 2003 and 2004 experienced 3 dust events each but in 2003 the events came in February and April, whereas in 2004 the events came in late April and mid-May. In 2005, of the 4 dust events, the first came in late March, the second and third in early April, and the fourth in early May. There are many similarities in trajectory patterns with some of these events. Preliminary analysis displays a few weather patterns bringing dust into the San Juan Mountains. The source of the dust will more than likely be from several locations with entrainment from source regions in SE Utah, N and NE Arizona, and extreme NW New Mexico. Moreover, winter and spring dust events may include intercontinental transport of dust from Asia.

Knudsen cell: Investigations about the uptake of important traces gases on ambient airborne mineral dust

NASA Astrophysics Data System (ADS)

Horn, Sabrina; Herrmann, Hartmut

2013-04-01

Mineral dust constitutes one of the largest mass fractions of natural aerosol. Its emission is estimated between 800 - 2000 Tg/a]. The dust is emitted through sand and dust storms in the arid regions of our planet, in particular by the great desserts such as the Sahara. The complex chemical composition of mineral dust is similar to crust material, because the dust is produced by soil erosion. The main components of mineral dust are SiO2 and Al2O3, whereas the active oxides (Fe2O3, TiO2) show some variety in content due to the dust source region. Mineral dust particles can be transported over several 1000 km and during its transport the surface can be changed by the uptake of water vapor and trace gases. On such modified surfaces homo- and heterogeneous reactions can occur. Trace gas uptakes play an important role in atmospheric chemistry as sinks or sources for several gaseous species. Hence, it is necessary to study these reactions. Among several experimental setups, the Knudsen cell is one of the promising tools to study reactive uptakes from the gas phase and the release of products formed by dust surface-mediated reactions. The Knudsen cell, implemented by Golden et al. in 1975, is a high vacuum flow reactor operating under molecular flow conditions, i.e., gas-wall collisions are highly preferred over gas-gas collisions. Despite several Knudsen cell studies examining the reaction between different traces gases and model dust surfaces constituted of not more than a few components, no measurements utilizing collected ambient mineral dust are done so far. For a better understanding of the chemistry on mineral dust surfaces gas uptake measurements will be done with a Knudsen cell. The first measurements are done with isopropanol on TiO2. Afterwards there are studies with different substrates like, Al2O3 (α- and γ-phase), FeO2, Arizona test dust, air collected mineral dust from the Cap Verde islands. In the beginning SO2, NO2 and HNO3 will be used.

Dust outpaces bedrock in nutrient supply to montane forest ecosystems

PubMed Central

Aciego, S. M.; Riebe, C. S.; Hart, S. C.; Blakowski, M. A.; Carey, C. J.; Aarons, S. M.; Dove, N. C.; Botthoff, J. K.; Sims, K. W. W.; Aronson, E. L.

2017-01-01

Dust provides ecosystem-sustaining nutrients to landscapes underlain by intensively weathered soils. Here we show that dust may also be crucial in montane forest ecosystems, dominating nutrient budgets despite continuous replacement of depleted soils with fresh bedrock via erosion. Strontium and neodymium isotopes in modern dust show that Asian sources contribute 18–45% of dust deposition across our Sierra Nevada, California study sites. The remaining dust originates regionally from the nearby Central Valley. Measured dust fluxes are greater than or equal to modern erosional outputs from hillslopes to channels, and account for 10–20% of estimated millennial-average inputs of bedrock P. Our results demonstrate that exogenic dust can drive the evolution of nutrient budgets in montane ecosystems, with implications for predicting forest response to changes in climate and land use. PMID:28348371

Understanding the Star Formation Process in the Filamentary Dark Cloud GF 9: Near-Infrared Observations

NASA Technical Reports Server (NTRS)

Ciardi, David R.; Woodward, Charles E.; Clemens, Dan P.; Harker, David E.; Rudy, Richard J.

1998-01-01

We have performed a near-infrared JHK survey of a dense core and a diffuse filament region within the filamentary dark cloud GF 9 (LDN 1082). The core region is associated with the IRAS point source PSC 20503+6006 and is suspected of being a site of star formation. The diffuse filament region has no associated IRAS point sources and is likely quiescent. We find that neither the core nor the filament region appears to contain a Class I or Class II young stellar object. As traced by the dust extinction, the core and filament regions contain 26 and 22 solar mass, respectively, with an average H2 volume density for both regions of approximately 2500/cu cm. The core region contains a centrally condensed extinction maximum with a peak extinction of A(sub v) greater than or approximately equal to 10 mag that appears to be associated with the IRAS point source. The average H2 volume density of the extinction core is approximately 8000/cu cm. The dust within the filament, however, shows no sign of a central condensation and is consistent with a uniform-density cylindrical distribution.

Chemical characterization of atmospheric dust from a weekly time series in the north Red Sea between 2006 and 2010

NASA Astrophysics Data System (ADS)

Torfstein, Adi; Teutsch, Nadya; Tirosh, Ofir; Shaked, Yeala; Rivlin, Tanya; Zipori, Assaf; Stein, Mordechai; Lazar, Boaz; Erel, Yigal

2017-08-01

Atmospheric dust loads and chemical compositions serve as a key link between global climate patterns and marine biogeochemical cycles. The primary source of atmospheric dust in the world today is the Sahara-Arabian desert belt. Although this source was also active during the Quaternary, the interpretation of paleo-dust records and their effects on marine ecosystems is complicated by the scarcely reported atmospheric load patterns of bioavailable phases (i.e., water and acid leachable phases) and present-day contamination of anthropogenic components. This study reports a multi-annual time series of atmospheric dust loads (2006-2016) and their chemical compositions (2006-2010) collected in the north Gulf of Aqaba (north Red Sea) at a weekly to bi-weekly resolution. Major and trace element abundances in each sample are reported for three fractions: water-soluble salts, carbonates and oxides (weak acid leach), and Al-silicates. Dust loads vary seasonally from low values in late summer (∼20-30 μg m-3) to higher values in the fall, and highest values in late winter and early spring (∼150-250 μg m-3). Major and trace element abundances allow to distinguish between the sources and chemical compositions that dominate high and low dust loads in each season. The water leachable fraction (L0) is relatively enriched in Na, Ca, K and Mg, the acid-leachable fraction (L1) is enriched in Ca as well as Na, Al, Mg, Zn, Cd and Pb, and the silicate residue (L2) in Al and Fe. High dust loads occurring mainly during winter and spring months are characterized by low Mg/Ca (L1, L2), low K/Al and Na/Al (L1) and high Ca/Al (L1), high Mg/Al (L2) and relatively un-weathered (L2) contents. High dust load intervals during winter months are characterized by low passing air masses originating from the Sahara, while the ambient winter dust (low dust load) is associated with proximal source regions from the East Sahara and Arabian Peninsula. During late winter and spring months, high dust loads originate from central and west Sahara and to a lesser extent from north Sahara. Low dust loads characterize the summer with limited compositional variability relative to winter-spring months. Summer dust is generally characterized by high K/Al (L1) ratios relative to late winter and spring. It is also relatively high in anthropogenic trace elements in the L0 and L1 fractions (e.g., Zn/Al, Pb/Al, Cr/Al, Ni/Al and V/Al), whereby back trajectories indicate the source of these components is primarily from south and east Europe. The total load (ng m-3) of anthropogenic trace elements however, remains higher during winter and spring, stemming from the overall significantly higher dust loads characterizing this time window. The temporal load patterns of important micronutrients such as Fe, Cd, Zn, Cu, Ni and others in the bio-available phases (L0, L1) are not correlated with major nutrients or Chlorophyll-a sea surface concentrations, suggesting that the atmospheric dust plays a limited role in driving primary productivity in the oligotrophic surface waters of the Gulf of Aqaba. On a wider scale, the results provide unique chemical fingerprinting of Sahara-Arabian dust that can be applied to reconstruct past trends in dust loads recorded in deep-sea cores and other geological archives from this and other regions.

Source apportionment of PM₁₀ and PM₂.₅ in a desert region in northern Chile.

PubMed

Jorquera, Héctor; Barraza, Francisco

2013-02-01

Estimating contributions of anthropogenic sources to ambient particulate matter (PM) in desert regions is a challenging issue because wind erosion contributions are ubiquitous, significant and difficult to quantify by using source-oriented, dispersion models. A receptor modeling analysis has been applied to ambient PM(10) and PM(2.5) measured in an industrial zone ~20 km SE of Antofagasta (23.63°S, 70.39°W), a midsize coastal city in northern Chile; the monitoring site is within a desert region that extends from northern Chile to southern Perú. Integrated 24-hour ambient samples of PM(10) and PM(2.5) were taken with Harvard Impactors; samples were analyzed by X Ray Fluorescence, ionic chromatography (NO(3)(-) and SO(4)(=)), atomic absorption (Na(+), K(+)) and thermal optical transmission for elemental and organic carbon determination. Receptor modeling was carried out using Positive Matrix Factorization (US EPA Version 3.0); sources were identified by looking at specific tracers, tracer ratios, local winds and wind trajectories computed from NOAA's HYSPLIT model. For the PM(2.5) fraction, six contributions were found - cement plant, 33.7 ± 1.3%; soil dust, 22.4 ± 1.6%; sulfates, 17.8 ± 1.7%; mineral stockpiles and brine plant, 12.4 ± 1.2%; Antofagasta, 8.5 ± 1.3% and copper smelter, 5.3 ± 0.8%. For the PM(10) fraction five sources were identified - cement plant, 38.2 ± 1.5%; soil dust, 31.2 ± 2.3%; mineral stockpiles and brine plant, 12.7 ± 1.7%; copper smelter, 11.5 ± 1.6% and marine aerosol, 6.5 ± 2.4%. Therefore local sources contribute to ambient PM concentrations more than distant sources (Antofagasta, marine aerosol) do. Soil dust is enriched with deposition of marine aerosol and calcium, sulfates and heavy metals from surrounding industrial activities. The mean contribution of suspended soil dust to PM(10) is 50 μg/m(3) and the peak daily value is 104 μg/m(3). For the PM(2.5) fraction, suspended soil dust contributes with an average of 9.3 μg/m(3) and a peak daily value of 31.5 μg/m(3). Copyright © 2012 Elsevier B.V. All rights reserved.

Kuiper Belt Dust Grains as a Source of Interplanetary Dust Particles

NASA Technical Reports Server (NTRS)

Liou, Jer-Chyi; Zook, Herbert A.; Dermott, Stanley F.

1996-01-01

The recent discovery of the so-called Kuiper belt objects has prompted the idea that these objects produce dust grains that may contribute significantly to the interplanetary dust population. In this paper, the orbital evolution of dust grains, of diameters 1 to 9 microns, that originate in the region of the Kuiper belt is studied by means of direct numerical integration. Gravitational forces of the Sun and planets, solar radiation pressure, as well as Poynting-Robertson drag and solar wind drag are included. The interactions between charged dust grains and solar magnetic field are not considered in the model. Because of the effects of drag forces, small dust grains will spiral toward the Sun once they are released from their large parent bodies. This motion leads dust grains to pass by planets as well as encounter numerous mean motion resonances associated with planets. Our results show that about 80% of the Kuiper belt grains are ejected from the Solar System by the giant planets, while the remaining 20% of the grains evolve all the way to the Sun. Surprisingly, the latter dust grains have small orbital eccentricities and inclinations when they cross the orbit of the Earth. This makes them behave more like asteroidal than cometary-type dust particles. This also enhances their chances of being captured by the Earth and makes them a possible source of the collected interplanetary dust particles; in particular, they represent a possible source that brings primitive/organic materials from the outer Solar System to the Earth. When collisions with interstellar dust grains are considered, however, Kuiper belt dust grains around 9 microns appear likely to be collisionally shattered before they can evolve toward the inner part of the Solar System. The collision destruction can be applied to Kuiper belt grains up to about 50 microns. Therefore, Kuiper belt dust grains within this range may not be a significant part of the interplanetary dust complex in the inner Solar System.

Changes in Stratiform Clouds of Mesoscale Convective Complex Introduced by Dust Aerosols

NASA Technical Reports Server (NTRS)

Lin, B.; Min, Q.-L.; Li, R.

2010-01-01

Aerosols influence the earth s climate through direct, indirect, and semi-direct effects. There are large uncertainties in quantifying these effects due to limited measurements and observations of aerosol-cloud-precipitation interactions. As a major terrestrial source of atmospheric aerosols, dusts may serve as a significant climate forcing for the changing climate because of its effect on solar and thermal radiation as well as on clouds and precipitation processes. Latest satellites measurements enable us to determine dust aerosol loadings and cloud distributions and can potentially be used to reduce the uncertainties in the estimations of aerosol effects on climate. This study uses sensors on various satellites to investigate the impact of mineral dust on cloud microphysical and precipitation processes in mesoscale convective complex (MCC). A trans-Atlantic dust outbreak of Saharan origin occurring in early March 2004 is considered. For the observed MCCs under a given convective strength, small hydrometeors were found more prevalent in the dusty stratiform regions than in those regions that were dust free. Evidence of abundant cloud ice particles in the dust regions, particularly at altitudes where heterogeneous nucleation of mineral dust prevails, further supports the observed changes of clouds and precipitation. The consequences of the microphysical effects of the dust aerosols were to shift the size spectrum of precipitation-sized hydrometeors from heavy precipitation to light precipitation and ultimately to suppress precipitation and increase the lifecycle of cloud systems, especially over stratiform areas.

Dust emissions from unpaved roads on the Colorado Plateau

NASA Astrophysics Data System (ADS)

Duniway, M.; Flagg, C.; Belnap, J.

2013-12-01

On the Colorado Plateau, elevated levels of aeolian dust have become a major land management and policy concern due to its influence on climate, weather, terrestrial ecosystem dynamics, landscape development and fertility, melting of snow and ice, air quality, and human health. Most desert soil surfaces are stabilized by plants, rocks, and/or physical or biological soil crusts, but once disturbed, sediment production from these surfaces can increase dramatically. Road development and use is a common surface disturbing activity in the region. The extent and density of roads and road networks is rapidly increasing due to continued energy exploration, infrastructure development, and off-highway recreation activities. Though it is well known that unpaved roads produce dust, the relative contribution of dust from existing roads or the implications of future road development to regional dust loading is unknown. To address this need, we have initiated a multifaceted research effort to evaluating dust emissions from unpaved roads regionally. At 34 sites arranged across various road surfaces and soil textures in southeastern Utah, we are: 1) monitoring dust emissions, local wind conditions, and vehicle traffic and 2) evaluating fugitive dust potential using a portable wind tunnel and measuring road characteristics that affect dust production. We will then 3) develop a GIS-based model that integrates results from 1 & 2 to estimate potential dust contributions from current and future scenarios of regional road development. Passive, horizontal sediment traps were installed at three distances downwind from the road edge. One control trap was placed upwind of the samplers to account for local, non-road dust emissions. An electronic vehicle counter and anemometer were also installed at monitoring sites. Dust samples were collected every three months at fixed heights, 15 cm up to 100 cm above the soil surface, from March 2010 to the present. Threshold friction velocities (TFV), the minimum wind velocity required to initiate erosion, and sediment production were also quantified using a portable wind tunnel at monitoring sites. Additionally, numerous characteristics including gravel cover, particle-size distribution, soil compaction, and loose-erodible material were measured on road surfaces at monitoring sites. Preliminary results suggest that roads are an important regional dust source, as emissions from roads are comparable to non-road, rural sources that are being monitored concurrently. While gravel roads produce more dust per day on average, per vehicle emissions are larger on dirt roads. Dust flux decreases with distance from the road edge on all road types, however this decline is less pronounced on dirt roads. Portable wind tunnel results indicate that TFV is consistently lower on dirt versus gravel roads across all soil types. Fugitive dust flux is generally larger and more variable on dirt roads compared to gravel roads. Initial analyses suggest that several easily measurable road surface characteristics can potentially be used to predict both TFV and sediment production, including: total gravel cover, gravel particle-size classes, clay content, and road compaction. The relation between TFV and total gravel cover in particular appears to be non-linear, with TFV increasing rapidly above ~40% gravel cover.

Global trends in visibility: Implications for dust sources

USGS Publications Warehouse

Mahowald, N.M.; Ballantine, J.A.; Feddema, J.; Ramankutty, N.

2007-01-01

There is a large uncertainty in the relative roles of human land use, climate change and carbon dioxide fertilization in changing desert dust source strength over the past 100 years, and the overall sign of human impacts on dust is not known. We used visibility data from meteorological stations in dusty regions to assess the anthropogenic impact on long term trends in desert dust emissions. Visibility data are available at thousands of stations globally from 1900 to the present, but we focused on 359 stations with more than 30 years of data in regions where mineral aerosols play a dominant role in visibility observations. We evaluated the 1974 to 2003 time period because most of these stations have reliable records only during this time. We first evaluated the visibility data against AERONET aerosol optical depth data, and found that only in dusty regions are the two moderately correlated. Correlation coefficients between visibility derived variables and AERONET optical depths indicate a moderate correlation (???0.47), consistent with capturing about 20% of the variability in optical depths. Two visibility derived variables appear to compare the best with AERONET observations: the fraction of observations with visibility less than 5 km (VIS5) and the surface extinction (EXT). Regional trends show that in many dusty places, VIS5 and EXT are statistically significantly correlated with the palmer drought severity index (based on precipitation and temperature) or surface wind speeds, consistent with dust temporal variability being largely driven by meteorology. This is especially true for North African and Chinese dust sources, but less true in the Middle East, Australia or South America, where there are not consistent patterns in the correlations. Climate indices such as El Nino or the North Atlantic Oscillation are not correlated with visibility derived variables in this analysis. There are few stations where visibility measures are correlated with cultivation or grazing estimates on a temporal basis, although this may be a function of the very coarse temporal resolution of the land use datasets. On the other hand, spatial analysis of the visibility data suggests that natural topographic lows are not correlated with visibility, but land use is correlated at a moderate level. This analysis is consistent with land use being important in some regions, but meteorology driving interannual variability during 1974-2003.

PM2.5 Source Apportionment: Reconciling Receptor Models for U.S. Nonurban and Urban Long-Term Networks.

PubMed

Chen, L-W Antony; Watson, John G; Chow, Judith C; DuBois, Dave W; Herschberger, Lisa

2011-11-01

Chemical mass balance (CMB) and trajectory receptor models were applied to speciated particulate matter with aerodynamic diameter ≤2.5 μm (PM 2.5 ) measurements from Speciation Trends Network (STN; part of the Chemical Speciation Network [CSN]) and Interagency Monitoring of Protected Visual Environments (IMPROVE) monitoring network across the state of Minnesota as part of the Minnesota PM 2.5 Source Apportionment Study (MPSAS). CMB equations were solved by the Unmix, positive matrix factorization (PMF), and effective variance (EV) methods, giving collective source contribution and uncertainty estimates. Geological source profiles developed from local dust materials were either incorporated into the EV-CMB model or used to verify factors derived from Unmix and PMF. Common sources include soil dust, calcium (Ca)-rich dust, diesel and gasoline vehicle exhausts, biomass burning, secondary sulfate, and secondary nitrate. Secondary sulfate and nitrate aerosols dominate PM 2.5 mass (50-69%). Mobile sources outweigh area sources at urban sites, and vice versa at rural sites due to traffic emissions. Gasoline and diesel contributions can be separated using data from the STN, despite significant uncertainties. Major differences between MPSAS and earlier studies on similar environments appear to be the type and magnitude of stationary sources, but these sources are generally minor (<7%) in this and other studies. Ensemble back-trajectory analysis shows that the lower Midwestern states are the predominant source region for secondary ammoniated sulfate in Minnesota. It also suggests substantial contributions of biomass burning and soil dust from out-of-state on occasions, although a quantitative separation of local and regional contributions was not achieved in the current study. Supplemental materials are available for this article. Go to the publisher's online edition of the Journal of the Air & Waste Management Association for a summary of input data, Unmix and PMF factor profiles, and additional maps. [Box: see text].

Monitoring An Intensive Dust Event over Northern China Using Multi-satellite Observation

NASA Astrophysics Data System (ADS)

She, L.; Xue, Y.; Guang, J.; Mei, L.; Che, Y.; Fan, C.; Xie, Y.

2017-12-01

The deserts in western/northern China are one of the major mineral dust source regions of the world. Large amount of dust are emitted and blown east and southeast, especially in spring. An intensive dust event occurred over Northern China during May 3 - 8, 2017. The dust storms came from deserts in China and Mongolia. Due to the long-distance transport, more than ten provinces were affected by this dust event, several provinces occurred strong dust storm. In this study, multi-satellite data were employed to analyse the spatial-temporal evolution and dynamic transport behaviour of the dust plume, especially the geostationary satellite data - Himawari8 Advanced Himawari Imager (AHI) data. AHI data was used to estimate hourly Aerosol Optical Depth (AOD) to monitoring the aerosol distribution as well as the dust plume movements, as the dust storms often characterized by high AOD. A simple dust index was also calculated based on AHI VIS and TIR data to estimate the dust intensity. Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data and the Ozone Monitoring Instrument (OMI) Aerosol Index were used as additional data sources to monitor the dust vertical distribution and provide independent information of dust presence. MODIS aerosol product and AERONET aerosol measurements were compared with the AHI retrieved AODs, the comparisons show a good agreement. The dust index was compared with the ground measurements as well as the corresponding RGB image. Simulations from HYSPLIT back-trajectory analysis shows similar temporal variation with the calculated AOD and dust index of the dust plume. Those comparisons with other satellite products and ground measurements suggested both the calculated AOD and dust index well depicted the dust events compared.

PMF and PSCF based source apportionment of PM2.5 at a regional background site in North China

NASA Astrophysics Data System (ADS)

Zong, Zheng; Wang, Xiaoping; Tian, Chongguo; Chen, Yingjun; Fu, Shanfei; Qu, Lin; Ji, Ling; Li, Jun; Zhang, Gan

2018-05-01

To apportion regional PM2.5 (atmospheric particles with aerodynamic diameter < 2.5 μm) source types and their geographic pattern in North China, 120 daily PM2.5 samples on Beihuangcheng Island (BH, a regional background site in North China) were collected from August 20th, 2014 to September 15th, 2015 showing one-year period. After the chemical analyses on carbonaceous species, water-soluble ions and inorganic elements, various approaches, such as Mann-Kendall test, chemical mass closure, ISORROPIA II model, Positive Matrix Factorization (PMF) linked with Potential Source Contribution Function (PSCF), were used to explore the PM2.5 speciation, sources, and source regions. Consequently, distinct seasonal variations of PM2.5 and its main species were found and could be explained by varying emission source characteristics. Based on PMF model, seven source factors for PM2.5 were identified, which were coal combustion + biomass burning, vehicle emission, mineral dust, ship emission, sea salt, industry source, refined chrome industry with the contribution of 48.21%, 30.33%, 7.24%, 6.63%, 3.51%, 3.2%, and 0.88%, respectively. In addition, PSCF analysis using the daily contribution of each factor from PMF result suggested that Shandong peninsula and Hebei province were identified as the high potential region for coal combustion + biomass burning; Beijing-Tianjin-Hebei (BTH) region was the main source region for industry source; Bohai Sea and East China Sea were found to be of high source potential for ship emission; Geographical region located northwest of BH Island was possessed of high probability for sea salt; Mineral dust presumably came from the region of Mongolia; Refined chrome industry mostly came from Liaoning, Jilin province; The vehicle emission was primarily of BTH region origin, centring on metropolises, such as Beijing and Tianjin. These results provided precious implications for PM2.5 control strategies in North China.

Meteorological aspects associated with dust storms in the Sistan region, southeastern Iran

NASA Astrophysics Data System (ADS)

Kaskaoutis, D. G.; Rashki, A.; Houssos, E. E.; Mofidi, A.; Goto, D.; Bartzokas, A.; Francois, P.; Legrand, M.

2015-07-01

Dust storms are considered natural hazards that seriously affect atmospheric conditions, ecosystems and human health. A key requirement for investigating the dust life cycle is the analysis of the meteorological (synoptic and dynamic) processes that control dust emission, uplift and transport. The present work focuses on examining the synoptic and dynamic meteorological conditions associated with dust-storms in the Sistan region, southeastern Iran during the summer season (June-September) of the years 2001-2012. The dust-storm days (total number of 356) are related to visibility records below 1 km at Zabol meteorological station, located near to the dust source. RegCM4 model simulations indicate that the intense northern Levar wind, the high surface heating and the valley-like characteristics of the region strongly affect the meteorological dynamics and the formation of a low-level jet that are strongly linked with dust exposures. The intra-annual evolution of the dust storms does not seem to be significantly associated with El-Nino Southern Oscillation, despite the fact that most of the dust-storms are related to positive values of Oceanic Nino Index. National Center for Environmental Prediction/National Center for Atmospheric Research reanalysis suggests that the dust storms are associated with low sea-level pressure conditions over the whole south Asia, while at 700 hPa level a trough of low geopotential heights over India along with a ridge over Arabia and central Iran is the common scenario. A significant finding is that the dust storms over Sistan are found to be associated with a pronounced increase of the anticyclone over the Caspian Sea, enhancing the west-to-east pressure gradient and, therefore, the blowing of Levar. Infrared Difference Dust Index values highlight the intensity of the Sistan dust storms, while the SPRINTARS model simulates the dust loading and concentration reasonably well, since the dust storms are usually associated with peaks in model simulations.

NMMB/BSC-DUST: model validation at regional scale in Northern Africa

NASA Astrophysics Data System (ADS)

Haustein, Karsten; Pérez, Carlos; Jorba, Oriol; María Baldasano, José; Janjic, Zavisa; Black, Tom; Slobodan, Nickovic; Prigent, Catherine; Laurent, Benoit

2010-05-01

While mineral dust distribution and effects are important at global scales, they strongly depend on dust emissions that are controlled on small spatial and temporal scales. Indeed, the accuracy of surface wind speed used in dust models is crucial. Due to the cubic higher-order power dependency on wind friction velocity and the threshold behaviour of dust emissions, small errors on surface wind speed lead to large dust emission errors. Most global dust models use prescribed wind fields provided by meteorological centres (e.g., NCEP and ECMWF) and their spatial resolution is currently never better than about 1°×1°. Such wind speeds tend to be strongly underestimated over large arid and semi-arid areas and do not account for reflect mesoscale character of systems responsible for a significant fraction of dust emissions regionally and globally. Other Another strong uncertainties in dust emissions from such approaches are related to the missrepresentation originates from of coarse representation of high subgrid-scale spatial heterogeneity in soil and vegetation boundary conditions, mainly in semi-arid areas. With the development of the new model NMMB-BSC/DUST [Pérez et al., 2008], we are now focusing on the evalution of the model sensitivity to several processes related to dust emissions. The results presented here are an intermediate step to provide global dust forecasts up to 7 days at sub-synoptic resolutions in the near future. NMMB-BSC/DUST is coupled online with the NOAA/NCEP/EMC global/regional NMMB atmospheric model [Janjic, 2005] extending from meso to global scales an being fully embedded into the Earth System Modeling Framework (ESMF). We performed regional simulations for the Northern African domain, including the Arabian peninsula and southern/central Europe (0 to 65°N and 25°W to 55°E) at 1/3°x1/3° and 1/6x1/6° horizontal resolution with 64 vertical layers. The model is initialized with 6-hourly updated NCEP 1x1° analysis data with a dust spin up of 5 days in advance. Dust columnal load, dust concentration at the surface, AOD and extinction coefficient are extracted for two time periods: March 2005 - corresponding with BoDEx campaign [Todd et al., 2008] - and May/June 2006 - corresponding with SAMUM I field campaign [Haustein et al., 2009]. Several model simulations were run with dust RRTM longwave and shortwave radiative feedback switched on or off, with dust vertical flux after Marticorena and Bergametti [1995] or after Alfaro and Gomez [2001], including viscous sublayer approach [Janjic, 1994] applied or not, and with or without preferential sources following Ginoux [2001]. Additionally, two new observational datasets of surface "aeolian" roughness length [Laurent, 2006; Prigent, 2005] are applied either for drag partition correction, or as substitution for the empirical model roughness length. These simulations are compared with detailed observational data. The atmospheric wind field is analyzed in terms of its capability to reproduce the low level jet in the Bodélé. References: Alfaro, S. C. and L. Gomes (2001). Modeling mineral aerosol production by eind erosion: Emission intensities and aerosol size distribution in source areas. Journal of Geophysical Research 106, D16, 18075-18084. Ginoux, P. et al. (2001). Sources and distribution of dust aerosols simulated with the GOCART model. J. Geophys. Res., 106, D17, 20255-20273. Haustein, K. et al. (2009). Regional dust model performance during SAMUM-I 2006. Geophysical Research Letters 36, L03812, doi:10.1029/2008GL036463. Janjic, Z. I. (1994). The Step-Mountain Eta Coordinate Model: Further Developments of the Convection, Viscous Sublayer, and Turbulence Closure Schemes. Monthly Weather Review 122, 927-945. Janjic, Z. I. (2005). A unified model approach from meso to global scales. Geophysical Research Abstracts 7, 05582, 2005, EGU05-A-05582. Laurent, B. Et al. (2006). Modeling mineral dust emissions from Chinese and Mongolian deserts. Global and Planetary Change 52, 121-141. Marticorena, B. and G. Bergametti (1995). Modeling the atmospheric dust cycle: 1. Design of a soil-derived dust emission scheme. Journal of Geophysical Research 100, D8, 16415-16430. Pérez, C. et al. (2008). An online mineral dust model within the global/regional NMMB: Current progress and plans. AGU Fall Meeting, 14-19 December 2008, San Francisco, USA. Prigent, C. et al. (2005). Estimation of aerodynamic roughness length in arid and semi-arid regions over the globe with the ERS scatterometer. Journal of Geophysical Research 110, D09205, doi:10.1029/2004JD005370. Todd, M. (2008). Quantifying uncertainty in estimates of mineral dust flux: An intercomparison of model performance over the Bodélé Depression, northern Chad. Journal of Geophysical Research 113, D24107, doi:10.1029/2008JD010476.

Spatial and temporal variability in desert dust and anthropogenic pollution in Iraq, 1997-2010.

PubMed

Chudnovsky, A Alexandra; Koutrakis, Petros; Kostinski, Alex; Proctor, Susan P; Garshick, Eric

2017-01-01

Satellite imaging has emerged as a method for monitoring regional air pollution and detecting areas of high dust concentrations. Unlike ground observations, continuous data monitoring is available with global coverage of terrestrial and atmospheric components. In this study we test the utility of different sources of satellite data to assess air pollution concentrations in Iraq. SeaWiFS and MODIS Deep Blue (DB) aerosol optical depth (AOD) products were evaluated and used to characterize the spatial and temporal pollution levels from the late 1990s through 2010. The AOD and Ångström exponent (an indicator of particle size, since smaller Ångström exponent values reflect a source that includes larger particles) were correlated on 50 × 50 km spatial resolution. Generally, AOD and Ångström exponent were inversely correlated, suggesting a significant contribution of coarse particles from dust storms to AOD maxima. Although the majority of grid cells exhibited this trend, a weaker relationship in other locations suggested an additional contribution of fine particles from anthropogenic sources. Tropospheric NO 2 densities from the OMI satellite were elevated over cities, also consistent with a contribution from anthropogenic sources. Our analysis demonstrates the use of satellite imaging data to estimate relative pollution levels and source contributions in areas of the world where direct measurements are not available. The authors demonstrated how satellite data can be used to characterize exposures to dust and to anthropogenic pollution for future health related studies. This approach is of a great potential to investigate the associations between subject-specific exposures to different pollution sources and their health effects in inaccessible regions and areas where ground monitoring is unavailable.

Spatial and temporal variability in desert dust and anthropogenic pollution in Iraq, 1997–2010

PubMed Central

Chudnovsky, A. Alexandra; Koutrakis, Petros; Kostinski, Alex; Proctor, Susan P.; Garshick, Eric

2016-01-01

Satellite imaging has emerged as a method for monitoring regional air pollution and detecting areas of high dust concentrations. Unlike ground observations, continuous data monitoring is available with global coverage of terrestrial and atmospheric components. In this study we test the utility of different sources of satellite data to assess air pollution concentrations in Iraq. SeaWiFS and MODIS Deep Blue (DB) aerosol optical depth (AOD) products were evaluated and used to characterize the spatial and temporal pollution levels from the late 1990s through 2010. The AOD and Ångström exponent (an indicator of particle size, since smaller Ångström exponent values reflect a source that includes larger particles) were correlated on 50 × 50 km spatial resolution. Generally, AOD and Ångström exponent were inversely correlated, suggesting a significant contribution of coarse particles from dust storms to AOD maxima. Although the majority of grid cells exhibited this trend, a weaker relationship in other locations suggested an additional contribution of fine particles from anthropogenic sources. Tropospheric NO2 densities from the OMI satellite were elevated over cities, also consistent with a contribution from anthropogenic sources. Our analysis demonstrates the use of satellite imaging data to estimate relative pollution levels and source contributions in areas of the world where direct measurements are not available. Implications The authors demonstrated how satellite data can be used to characterize exposures to dust and to anthropogenic pollution for future health related studies. This approach is of a great potential to investigate the associations between subject-specific exposures to different pollution sources and their health effects in inaccessible regions and areas where ground monitoring is unavailable. PMID:28001122

Periodic input of dust over the Eastern Carpathians during the Holocene linked with Saharan desertification and human impact

NASA Astrophysics Data System (ADS)

Longman, Jack; Veres, Daniel; Ersek, Vasile; Salzmann, Ulrich; Hubay, Katalin; Bormann, Marc; Wennrich, Volker; Schäbitz, Frank

2017-07-01

Reconstructions of dust flux have been used to produce valuable global records of changes in atmospheric circulation and aridity. These studies have highlighted the importance of atmospheric dust in marine and terrestrial biogeochemistry and nutrient cycling. By investigating a 10 800-year-long paleoclimate archive from the Eastern Carpathians (Romania) we present the first peat record of changing dust deposition over the Holocene for the Carpathian-Balkan region. Using qualitative (X-ray fluorescence (XRF) core scanning) and quantitative inductively coupled plasma optical emission spectrometer(ICP-OES) measurements of lithogenic (K, Si, Ti) elements, we identify 10 periods of major dust deposition between 9500-9200, 8400-8100, 7720-7250, 6350-5950, 5450-5050, 4130-3770, 3450-2850, 2000-1450, 800-620, and 60 cal yr BP to present. In addition, we used testate amoeba assemblages preserved within the peat to infer local palaeohydroclimatic conditions. Our record highlights several discrepancies between eastern and western European dust depositional records and the impact of highly complex hydrological regimes in the Carpathian region. Since 6100 cal yr BP, we find that the geochemical indicators of dust flux have become uncoupled from the local hydrology. This coincides with the appearance of millennial-scale cycles in the dust input and changes in geochemical composition of dust. We suggest that this is indicative of a shift in dust provenance from local-regional (likely loess-related) to distal (Saharan) sources, which coincide with the end of the African Humid Period and the onset of Saharan desertification.

The potential influence of Asian and African mineral dust on ice, mixed-phase and liquid water clouds

NASA Astrophysics Data System (ADS)

Wiacek, A.; Peter, T.; Lohmann, U.

2010-09-01

This modelling study explores the availability of mineral dust particles as ice nuclei for interactions with ice, mixed-phase and liquid water clouds, also tracking the particles' history of cloud-processing. We performed 61 320 one-week forward trajectory calculations originating near the surface of major dust emitting regions in Africa and Asia using high-resolution meteorological analysis fields for the year 2007. Dust-bearing trajectories were assumed to be those coinciding with known dust emission seasons, without explicitly modelling dust emission and deposition processes. We found that dust emissions from Asian deserts lead to a higher potential for interactions with high ice clouds, despite being the climatologically much smaller dust emission source. This is due to Asian regions experiencing significantly more ascent than African regions, with strongest ascent in the Asian Taklimakan desert at ~25%, ~40% and 10% of trajectories ascending to 300 hPa in spring, summer and fall, respectively. The specific humidity at each trajectory's starting point was transported in a Lagrangian manner and relative humidities with respect to water and ice were calculated in 6-h steps downstream, allowing us to estimate the formation of liquid, mixed-phase and ice clouds. Downstream of the investigated dust sources, practically none of the simulated air parcels reached conditions of homogeneous ice nucleation (T≲-40 °C) along trajectories that have not experienced water saturation first. By far the largest fraction of cloud forming trajectories entered conditions of mixed-phase clouds, where mineral dust will potentially exert the biggest influence. The majority of trajectories also passed through atmospheric regions supersaturated with respect to ice but subsaturated with respect to water, where so-called "warm ice clouds" (T≳-40 °C) theoretically may form prior to supercooled water or mixed-phase clouds. The importance of "warm ice clouds" and the general influence of dust in the mixed-phase cloud region are highly uncertain due to both a considerable scatter in recent laboratory data from ice nucleation experiments, which we briefly review in this work, and due to uncertainties in sub-grid scale vertical transport processes unresolved by the present trajectory analysis. For "classical" cirrus-forming temperatures (T≲-40 °C), our results show that only mineral dust ice nuclei that underwent mixed-phase cloud-processing, most likely acquiring coatings of organic or inorganic material, are likely to be relevant. While the potential paucity of deposition ice nuclei shown in this work dimishes the possibility of deposition nucleation, the absence of liquid water droplets at T≲-40 °C makes the less explored contact freezing mechanism (involving droplet collisions with bare ice nuclei) highly inefficient. These factors together indicate the necessity of further systematic studies of immersion mode ice nucleation on mineral dust suspended in atmospherically relevant coatings.

Characterization of Dust Properties Near Source Region During ACE-Asia: A Column Satellite-Surface Perspective

NASA Technical Reports Server (NTRS)

Tsay, S. -C.; Ji, Q.; Chu, A.; Hsu, C.; Holben, B.; Campbell, J.; Welton, E. J.; Shu, P. K.

2002-01-01

Many recent field experiments are designed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentrations over eastern/southeastern Asia and along the rim of the western Pacific. For example, the ACE-Asia was conducted from March-May 2001 in the vicinity of the Taklimakan and Gobi deserts, East Coast of China, Yellow Sea, Korea, and Japan, along the pathway of Kosa (severe events that blanket East Asia with yellow desert dust, peaked in the Spring season). Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian aerosols is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia we have measured continuously aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over homogeneous areas from surface. The inclusion of flux measurements permits the determination of aerosol radiative flux in addition to measurements of loading and optical depth. At the time of the Terra/MODIS, SeaWiFS, TOMS and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. Preliminary results will be presented and discussed their implications in regional climatic effects.

Colorado air quality impacted by long-range-transported aerosol: a set of case studies during the 2015 Pacific Northwest fires

NASA Astrophysics Data System (ADS)

Creamean, Jessie M.; Neiman, Paul J.; Coleman, Timothy; Senff, Christoph J.; Kirgis, Guillaume; Alvarez, Raul J.; Yamamoto, Atsushi

2016-09-01

Biomass burning plumes containing aerosols from forest fires can be transported long distances, which can ultimately impact climate and air quality in regions far from the source. Interestingly, these fires can inject aerosols other than smoke into the atmosphere, which very few studies have evidenced. Here, we demonstrate a set of case studies of long-range transport of mineral dust aerosols in addition to smoke from numerous fires (including predominantly forest fires and a few grass/shrub fires) in the Pacific Northwest to Colorado, US. These aerosols were detected in Boulder, Colorado, along the Front Range using beta-ray attenuation and energy-dispersive X-ray fluorescence spectroscopy, and corroborated with satellite-borne lidar observations of smoke and dust. Further, we examined the transport pathways of these aerosols using air mass trajectory analysis and regional- and synoptic-scale meteorological dynamics. Three separate events with poor air quality and increased mass concentrations of metals from biomass burning (S and K) and minerals (Al, Si, Ca, Fe, and Ti) occurred due to the introduction of smoke and dust from regional- and synoptic-scale winds. Cleaner time periods with good air quality and lesser concentrations of biomass burning and mineral metals between the haze events were due to the advection of smoke and dust away from the region. Dust and smoke present in biomass burning haze can have diverse impacts on visibility, health, cloud formation, and surface radiation. Thus, it is important to understand how aerosol populations can be influenced by long-range-transported aerosols, particularly those emitted from large source contributors such as wildfires.

Synoptic-scale dust transport events in the southern Himalaya

NASA Astrophysics Data System (ADS)

Duchi, R.; Cristofanelli, P.; Marinoni, A.; Bourcier, L.; Laj, P.; Calzolari, F.; Adhikary, B.; Verza, G. P.; Vuillermoz, E.; Bonasoni, P.

2014-06-01

The variability of long-range dust transport events observed in the southern Himalaya and its relation with source areas have been studied thanks to five years’ continuous measurements which were carried out at the “Nepal Climate Observatory-Pyramid” (NCO-P, 27°57‧N, 86°48‧E), the highest Northern Hemisphere GAW-WMO global station sited at 5079 m a.s.l. in the high Khumbu valley (Nepal) on the southern Himalaya. During the period March 2006-February 2011, the analyses of the aerosol particle concentrations and LAGRANTO three-dimensional backward trajectories indicated the occurrence of 275 days affected by synoptic-scale dust transport, which account for 22.2% of the investigated period. The frequency of dust transport days (DTDs) showed a clear seasonal cycle, with the highest seasonal value observed during pre-monsoon season (33.5% of the pre-monsoon’s days are DTDs). Large enhancements in coarse aerosol number concentration N1-10 (average: +689%) and mass PM1-10 (average: +1086%) were observed during the dust transport events as compared to the days without dust (dust-free days, DFDs). In addition, the single scattering albedo (SSA) also showed higher values, ranging from 0.87 to 0.90, during DTDs with respect to DFDs (0.80-0.87). The predominant source of mineral dust reaching the measurement site was identified in the arid regions of the north-western Indian subcontinent (Thar desert), which accounted for 41.6% of the trajectories points associated with DTDs. Seasonal analysis also indicated that the winter season was significantly influenced by far western desert regions, such as North Africa and the Arabic Peninsula.

Transpacific Transport of Dust to North American High-Elevation Sites: Integrated Dataset and Model Outputs

NASA Astrophysics Data System (ADS)

Kassianov, E.; Pekour, M. S.; Flynn, C. J.; Berg, L. K.; Beranek, J.; Zelenyuk, A.; Zhao, C.; Leung, L. R.; Ma, P. L.; Riihimaki, L.; Fast, J. D.; Barnard, J.; Hallar, G. G.; McCubbin, I.; Eloranta, E. W.; McComiskey, A. C.; Rasch, P. J.

2017-12-01

Understanding the effects of dust on the regional and global climate requires detailed information on particle size distributions and their changes with distance from the source. Awareness is now growing about the tendency of the dust coarse mode with moderate ( 3.5 µm) volume median diameter (VMD) to be rather insensitive to complex removal processes associated with long-range transport of dust from the main sources. Our study, with a focus on the transpacific transport of dust, demonstrates that the impact of coarse mode aerosol (VMD 3µm) is well defined at the high-elevation mountain-top Storm Peak Laboratory (SPL, about 3.2 km MSL) and nearby Atmospheric Radiation Measurement (ARM) Climate Research Facility Mobile Facility (AMF) during March 2011. Significant amounts of coarse mode aerosol are also found at the nearest Aerosol Robotic Network (AERONET) site. Outputs from the high-resolution Weather Research and Forecasting (WRF) Model coupled with chemistry (WRF-Chem) show that the major dust event is likely associated with transpacific transport of Asian and African plumes. Satellite data, including the Moderate Resolution Imaging Spectroradiometer (MODIS) and Multiangle Imaging SpectroRadiometer (MISR) aerosol optical depth (AOD) and plume height from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) lidar data provide the observational support of the WRF-Chem simulations. Our study complements previous findings by indicating that the quasi-static nature of the coarse mode appears to be a reasonable approximation for Asian and African dust despite expected frequent orographic precipitation over mountainous regions in the western United States.

Climate change and climate systems influence and control the atmospheric dispersion of desert dust: implications for human health

USGS Publications Warehouse

Griffin, Dale W.; Ragaini, Richard C.

2010-01-01

The global dispersion of desert dust through Earth’s atmosphere is greatly influenced by temperature. Temporal analyses of ice core data have demonstrated that enhanced dust dispersion occurs during glacial events. This is due to an increase in ice cover, which results in an increase in drier terrestrial cover. A shorter temporal analysis of dust dispersion data over the last 40 years has demonstrated an increase in dust transport. Climate systems or events such as the North Atlantic Oscillation, the Indian Ocean subtropical High, Pacific Decadal Oscillation, and El Nino-Sothern Oscillation are known to influence global short-term dust dispersion occurrence and transport routes. Anthropogenic influences on dust transport include deforestation, harmful use of topsoil for agriculture as observed during the American Dust Bowl period, and the creation of dry seas (Aral Sea) and lakes (Lake Owens in California and Lake Chad in North Africa) through the diversion of source waters (for irrigation and drinking water supplies). Constituents of desert dust both from source regions (pathogenic microorganisms, organic and inorganic toxins) and those scavenged through atmospheric transport (i.e., industrial and agricultural emissions) are known to directly impact human and ecosystem health. This presentation will present a review of global scale dust storms and how these events can be both a detriment and benefit to various organisms in downwind environments.

Comparing dust flux records from the Subarctic North Pacific and Greenland: Implications for atmospheric transport to Greenland and for the application of dust as a chronostratigraphic tool

NASA Astrophysics Data System (ADS)

Serno, Sascha; Winckler, Gisela; Anderson, Robert F.; Maier, Edith; Ren, Haojia; Gersonde, Rainer; Haug, Gerald H.

2015-06-01

We present a new record of eolian dust flux to the western Subarctic North Pacific (SNP) covering the past 27,000 years based on a core from the Detroit Seamount. Comparing the SNP dust record to the North Greenland Ice Core Project (NGRIP) ice core record shows significant differences in the amplitude of dust changes to the two regions during the last deglaciation, while the timing of abrupt changes is synchronous. If dust deposition in the SNP faithfully records its mobilization in East Asian source regions, then the difference in the relative amplitude must reflect climate-related changes in atmospheric dust transport to Greenland. Based on the synchronicity in the timing of dust changes in the SNP and Greenland, we tie abrupt deglacial transitions in the 230Th-normalized 4He flux record to corresponding transitions in the well-dated NGRIP dust flux record to provide a new chronostratigraphic technique for marine sediments from the SNP. Results from this technique are complemented by radiocarbon dating, which allows us to independently constrain radiocarbon paleoreservoir ages. We find paleoreservoir ages of 745 ± 140 years at 11,653 year B.P., 680 ± 228 years at 14,630 year B.P., and 790 ± 498 years at 23,290 year B.P. Our reconstructed paleoreservoir ages are consistent with modern surface water reservoir ages in the western SNP. Good temporal synchronicity between eolian dust records from the Subantarctic Atlantic and equatorial Pacific and the ice core record from Antarctica supports the reliability of the proposed dust tuning method to be used more widely in other global ocean regions.

Experimental Study of Lunar Dust Transportation due to Electrostatic Forces and Micro-meteorite Impacts

NASA Astrophysics Data System (ADS)

Orger, N. C.; Toyoda, K.; Cho, M.

2017-12-01

Lunar dust particles can be transported via several physical mechanisms above the surface, and the electrostatic dust lofting was suspected to be the responsible mechanism for the high-altitude lunar horizon glow above the terminator region. Most of the recent studies have shown that contact forces acting on the dust grains of sub-micrometer and micrometer sizes are much larger than the electrostatic forces resulting from the ambient plasma conditions; however, the electrostatic forces are strong enough to accelerate the lunar dust grains to high altitudes once the dust particles are separated from the surface by an initial mechanism. In this study our purpose is to investigate if the dust particles can be transported under the electrostatic forces after they are released from the surface by the micrometeorite impacts. It is expected to be the most of the dust grains will be launched from the elastic deformation regions, and the contact forces will be canceled after they are moved tens of nanometers. For the experiments, silica particles are used in a cavity with 2 cm diameter and 5 mm depth on the graphite plates. First, the dust particles are baked under an infrared lamp to release the absorbed atmospheric particles in the vacuum chamber. Second, the electron beam source emits electrons with 100 - 200 eV energies, and a Faraday cup measures the electron current in the vacuum chamber. Third, a laser beam is used to simulate micro-meteorite impacts, and the results are monitored with a high speed camera mostly focusing on the elastic deformation region. Therefore, this study investigates how the impacts modify the dust transportation as an initial mechanism for electrostatic dust lofting to high altitudes.

Role of Surface Wind and Vegetation Cover in Multi-decadal Variations of Dust Emission in the Sahara and Sahel

NASA Technical Reports Server (NTRS)

Kim, Dong; Chin, Mian; Remer, Lorraine A.; Diehl, Thomas L.; Bian, Huisheng; Yu, Hongbin; Brown, Molly E.; Stockwell, William R.

2016-01-01

North Africa, the world's largest dust source, is non-uniform, consisting of a permanently arid region (Sahara), a semi-arid region (Sahel), and a relatively moist vegetated region (Savanna), each with very different rainfall patterns and surface conditions. This study aims to better understand the controlling factors that determine the variation of dust emission in North Africa over a 27-year period from 1982 to 2008, using observational data and model simulations. The results show that the model-derived Saharan dust emission is only correlated with the 10-m winds (W10m) obtained from reanalysis data, but the model-derived Sahel dust emission is correlated with both W10m and the Normalized Difference Vegetation Index (NDVI) that is obtained from satellite. While the Saharan dust accounts for 82 of the continental North Africa dust emission (1340-1570 Tg year(exp -1) in the 27-year average, the Sahel accounts for 17 with a larger seasonal and inter-annual variation (230-380 Tg year(exp -1), contributing about a quarter of the transatlantic dust transported to the northern part of South America. The decreasing dust emission trend over the 27-year period is highly correlated with W10m over the Sahara (R equals 0.92). Over the Sahel, the dust emission is correlated with W10m (R 0.69) but is also anti-correlated with the trend of NDVI (R equals 0.65). W10m is decreasing over both the Sahara and the Sahel between 1982 and 2008, and the trends are correlated (R equals 0.53), suggesting that Saharan Sahelian surface winds are a coupled system, driving the inter-annual variation of dust emission.

Use of MODIS Satellite Data to Evaluate Juniperus spp. Pollen Phenology to Support a Pollen Dispersal Model, PREAM, to Support Public Health Allergy Alerts

NASA Technical Reports Server (NTRS)

Luvall, J. C.; Sprigg, W. A.; Levetin, E.; Huete, A.; Nickovic, S.; Prasad, A.; Pejanovic, G. A.; Vukovic, A.; VandeWater, P. K.; Budge, A. M.;

Use of MODIS Satellite Data to Evaluate Juniperus spp. Pollen Phenology to Support a Pollen Dispersal Model, PREAM, to Support Public Health Allergy Alerts

NASA Technical Reports Server (NTRS)

Luvall, J. C.; Sprigg, W. A.; Levetin, E.; Huete, A.; Nickovic, S.; Prasad, A.; Pejanovic, G. A.; Vukovic, A.; VandeWater, P. K.; Budge, A. M.;

Use of MODIS Satellite Data to Evaluate Juniperus spp. Pollen Phenology to Support a Pollen Dispersal Model, PREAM, to Support Public Health Allergy Alerts

NASA Astrophysics Data System (ADS)

Luvall, J. C.; Sprigg, W. A.; Levetin, E.; Huete, A. R.; Nickovic, S.; Prasad, A. K.; Pejanovic, G.; Vukovic, A.; Van De Water, P. K.; Budge, A.; Hudspeth, W. B.; Krapfl, H.; Toth, B.; Zelicoff, A.; Myers, O.; Bunderson, L.; Ponce-Campos, G.; Menache, M.; Crimmins, T. M.; Vujadinovic, M.

2012-12-01

Pollen can be transported great distances. Van de Water et. al., 2003 reported Juniperus spp. pollen was transported 200-600 km. Hence local observations of plant phenology may not be consistent with the timing and source of pollen collected by pollen sampling instruments. The DREAM (Dust REgional Atmospheric Model, Nickovic et al. 2001) is a verified model for atmospheric dust transport modeling using MODIS data products to identify source regions and concentrations of dust. We are modifying the DREAM model to incorporate pollen transport. Pollen emission is based on MODIS-derived phenology of Juniperus spp. communities. Ground-based observational records of pollen release timing and quantities will be used as model verification. This information will be used to support the Centers for Disease Control and Prevention's National Environmental Public Health Tracking Program and the State of New Mexico environmental public health decision support for asthma and allergies alerts.

Exploring the variability of aerosol particle composition in the Arctic: a study from the springtime ACCACIA campaign

NASA Astrophysics Data System (ADS)

Young, G.; Jones, H. M.; Darbyshire, E.; Baustian, K. J.; McQuaid, J. B.; Bower, K. N.; Connolly, P. J.; Gallagher, M. W.; Choularton, T. W.

2015-10-01

Single-particle compositional analysis of filter samples collected on-board the FAAM BAe-146 aircraft is presented for six flights during the springtime Aerosol-Cloud Coupling and Climate Interactions in the Arctic (ACCACIA) campaign (March-April 2013). Scanning electron microscopy was utilised to derive size distributions and size-segregated particle compositions. These data were compared to corresponding data from wing-mounted optical particle counters and reasonable agreement between the calculated number size distributions was found. Significant variability in composition was observed, with differing external and internal mixing identified, between air mass trajectory cases based on HYSPLIT analyses. Dominant particle classes were silicate-based dusts and sea salts, with particles notably rich in K and Ca detected in one case. Source regions varied from the Arctic Ocean and Greenland through to northern Russia and the European continent. Good agreement between the back trajectories was mirrored by comparable compositional trends between samples. Silicate dusts were identified in all cases, and the elemental composition of the dust was consistent for all samples except one. It is hypothesised that long-range, high-altitude transport was primarily responsible for this dust, with likely sources including the Asian arid regions.

Modelling the diffuse dust emission around Orion

NASA Astrophysics Data System (ADS)

Saikia, Gautam; Shalima, P.; Gogoi, Rupjyoti

2018-06-01

We have studied the diffuse radiation in the surroundings of M42 using photometric data from the Galaxy Evolution Explorer (GALEX) in the far-ultraviolet (FUV) and infrared observations of the AKARI space telescope. The main source of the FUV diffuse emission is the starlight from the Trapezium stars scattered by dust in front of the nebula. We initially compare the diffuse FUV with the far-infrared (FIR) observations at the same locations. The FUV-IR correlations enable us to determine the type of dust contributing to this emission. We then use an existing model for studying the FUV dust scattering in Orion to check if it can be extended to regions away from the centre in a 10 deg radius. We obtain an albedo, α = 0.7 and scattering phase function asymmetry factor, g = 0.6 as the median values for our dust locations on different sides of the central Orion region. We find a uniform value of optical parameters across our sample of locations with the dust properties varying significantly from those at the centre of the nebula.

The energetics and mass structure of regions of star formation: S201

NASA Technical Reports Server (NTRS)

Thronson, H. A., Jr.; Smith, H. A.; Lada, C. J.; Glaccum, W.; Harper, D. A.; Loewenstein, R. F.; Smith, J.

1984-01-01

Theoretical predictions about dust and gas in star forming regions are tested by observing a 4 arcmin region surrounding the radio continuum source in 5201. The object was mapped in two far infrared wavelengths and found to show significant extended emission. Under the assumption that the molecular gas is heated solely via thermal coupling with the dust, the volume density was mapped in 5201. The ratios of infrared optical depth to CO column density were calculated for a number of positions in the source. Near the center of the cloud the values are found to be in good agreement with other determinations for regions with lower column density. In addition, the observations suggest significant molecular destruction in the outer parts of the object. Current models of gas heating were used to calculate a strong limit for the radius of the far infrared emitting grains, equal to or less than 0.15 micron. Grains of about this size are required by the observation of high temperature (T equal to or greater than 20 K) gas in many sources.

A study of impact of Asian dusts and their transport pathways to Hong Kong using multiple AERONET data, trajectory, and in-situ measurements

NASA Astrophysics Data System (ADS)

Wong, Man Sing; Nichol, Janet Elizabeth; Lee, Kwon Ho

2010-10-01

Hong Kong, a commercial and financial city located in south-east China has suffered serious air pollution for the last decade due largely to rapid urban and industrial expansion of the cities of mainland China. However, the potential sources and pathways of aerosols transported to Hong Kong have not been well researched due to the lack of air quality monitoring stations in southern China. Here, an integrated method combining the AErosol RObotic NETwork (AERONET) data, trajectory and Potential Source Contribution Function (PSCF) modeling is used to identify the potential transport pathways and contribution of sources from four characteristic aerosol types. Four characteristic aerosol types were defined using a total of 730 AERONET data measurements between 2005 and 2008. They are coastal urban, polluted urban, dust (likely to be long distance desert dust), and heavy pollution. Results show that the sources of polluted urban and heavy pollution are associated with industrial emissions in southern China, whereas coastal urban aerosols have been affected both from natural marine aerosol and emissions. The PSCF map of dust shows a wide range of pathways followed by east- and south-eastwards trajectories from northwest China to Hong Kong. Although the contribution from dust sources is small compared to the anthropogenic aerosols, a serious recent dust outbreak has been observed in Hong Kong with an elevation of the Air Pollution Index to 500, compared with 50-100 on normal days. Therefore, the combined use of clustered AERONET data, trajectory and the PSCF models can help to resolve the longstanding issue about source regions and characteristics of pollutants carried to Hong Kong.

The potential influence of Asian and African mineral dust on ice, mixed-phase and liquid water clouds

NASA Astrophysics Data System (ADS)

Wiacek, A.; Peter, T.; Lohmann, U.

2010-02-01

This modelling study explores the availability of mineral dust particles as ice nuclei for interactions with ice, mixed-phase and liquid water clouds, also tracking the particles' history of cloud-processing. We performed 61 320 one-week forward trajectory calculations originating near the surface of major dust emitting regions in Africa and Asia using high-resolution meteorological analysis fields for the year 2007. Without explicitly modelling dust emission and deposition processes, dust-bearing trajectories were assumed to be those coinciding with known dust emission seasons. We found that dust emissions from Asian deserts lead to a higher potential for interactions with high clouds, despite being the climatologically much smaller dust emission source. This is due to Asian regions experiencing significantly more ascent than African regions, with strongest ascent in the Asian Taklimakan desert at ~25%, ~40% and 10% of trajectories ascending to 300 hPa in spring, summer and fall, respectively. The specific humidity at each trajectory's starting point was transported in a Lagrangian manner and relative humidities with respect to water and ice were calculated in 6-h steps downstream, allowing us to estimate the formation of liquid, mixed-phase and ice clouds. Practically none of the simulated air parcels reached regions where homogeneous ice nucleation can take place (T≲-40 °C) along trajectories that have not experienced water saturation first. By far the largest fraction of cloud forming trajectories entered conditions of mixed-phase clouds, where mineral dust will potentially exert the biggest influence. The majority of trajectories also passed through regions supersaturated with respect to ice but subsaturated with respect to water, where "warm" (T≳-40 °C) ice clouds may form prior to supercooled water or mixed-phase clouds. The importance of "warm" ice clouds and the general influence of dust in the mixed-phase cloud region are highly uncertain due to considerable scatter in recent laboratory data from ice nucleation experiments, which we briefly review in this work. For "classical" cirrus-forming temperatures, our results show that only mineral dust IN that underwent mixed-phase cloud-processing previously are likely to be relevant, and, therefore, we recommend further systematic studies of immersion mode ice nucleation on mineral dust suspended in atmospherically relevant coatings.

Mid-troposphere transport of Middle-East dust over the Arabian Sea and its effect on rainwater composition and sensitive ecosystems over India.

PubMed

Ramaswamy, V; Muraleedharan, P M; Babu, C Prakash

2017-10-20

The importance of mineral dust and aerosols in the transfer of bio-essential elements to terrestrial and marine ecosystems far removed from the source region is well known. Aerosol concentrations measured at the surface over the west coast of India during the SW monsoon period (June to September) are usually very low as pristine maritime air from the Southern Indian Ocean blows over this region. However, we find very high levels of mineral dust and dust derived nutrients in rainwater collected during the SW monsoon period. We show that the dry, warm and dusty Red Sea Wind and Shamal Wind from the Middle-East override the moist oceanic Low-Level Jet (Findlater Jet) of the SW monsoon and transport large quantities of dust at heights between 2 km and 5 km over the Indian Peninsula. A substantial portion is the desert dust is scavenged and wet-deposited over the Western Ghats of India where it neutralizes the acidity of rainwater and provides substantial amounts of nutrients that have the potential to impact sensitive ecosystems in this region. After the Red Sea and Shamal Winds subside in September, the alkaline rainwater reverts to the acidic range due to soluble ions derived from local carbonaceous aerosols.

Probing the interstellar dust towards the Galactic Centre: dust-scattering halo around AX J1745.6-2901

NASA Astrophysics Data System (ADS)

Jin, Chichuan; Ponti, Gabriele; Haberl, Frank; Smith, Randall

2017-07-01

AX J1745.6-2901 is an X-ray binary located at only 1.45 arcmin from Sgr A⋆, showcasing a strong X-ray dust-scattering halo. We combine Chandra and XMM-Newton observations to study the halo around this X-ray binary. Our study shows two major thick dust layers along the line of sight (LOS) towards AX J1745.6-2901. The LOS position and NH of these two layers depend on the dust grain models with different grain size distributions and abundances. But for all the 19 dust grain models considered, dust layer-1 is consistently found to be within a fractional distance of 0.11 (mean value: 0.05) to AX J1745.6-2901 and contains only (19-34) per cent (mean value: 26 per cent) of the total LOS dust. The remaining dust is contained in layer-2, which is distributed from the Earth up to a mean fractional distance of 0.64. A significant separation between the two layers is found for all the dust grain models, with a mean fractional distance of 0.31. Besides, an extended wing component is discovered in the halo, which implies a higher fraction of dust grains with typical sizes ≲590 Å than considered in current dust grain models. Assuming AX J1745.6-2901 is 8 kpc away, dust layer-2 would be located in the Galactic disc several kpc away from the Galactic Centre (GC). The dust scattering halo biases the observed spectrum of AX J1745.6-2901 severely in both spectral shape and flux, and also introduces a strong dependence on the size of the instrumental point spread function and the source extraction region. We build xspec models to account for this spectral bias, which allow us to recover the intrinsic spectrum of AX J1745.6-2901 free from dust-scattering opacity. If dust layer-2 also intervenes along the LOS to Sgr A⋆ and other nearby GC sources, a significant spectral correction for the dust-scattering opacity would be necessary for all these GC sources.

Characterization of potential zones of dust generation at eleven stations in the southern Sahara

NASA Astrophysics Data System (ADS)

Clark, I.; Assamoi, P.; Bertrand, J.; Giorgi, F.

Synoptic wind data for multi-decadal periods at eleven stations located in the southern Sahara region (Agadez, Atar, Bilma, Dori, Gao, Kayes, Nema, Niamey, Nouadhibou, Ouagadougou and Tessalit) are used to study the monthly dust deflation power over the region. We found that, regardless of the conditions of the soil, the deflation power (or wind efficiency) is not sufficient to generate significant amounts of aerosols south of 15°N. North of this latitude, the deflation power is much larger, with potential zones of either very strong deflation (Nouadhibou and Bilma) or severe deflation (Gao, Tessalit, Nema, Atar, Agadez). Stations in the Sahel region such as Gao, Agadez and Tessalit are characterized by a gradual reinforcement of the deflation power between 1970 and 1984 in correspondence of increasing desertification over the region. During this same period, Bilma, a well know region of dust source, experienced a major reduction in deflation power due to shifts in large scale wind patterns.

DECONVOLUTION OF IMAGES FROM BLAST 2005: INSIGHT INTO THE K3-50 AND IC 5146 STAR-FORMING REGIONS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Roy, Arabindo; Netterfield, Calvin B.; Ade, Peter A. R.

2011-04-01

We present an implementation of the iterative flux-conserving Lucy-Richardson (L-R) deconvolution method of image restoration for maps produced by the Balloon-borne Large Aperture Submillimeter Telescope (BLAST). Compared to the direct Fourier transform method of deconvolution, the L-R operation restores images with better-controlled background noise and increases source detectability. Intermediate iterated images are useful for studying extended diffuse structures, while the later iterations truly enhance point sources to near the designed diffraction limit of the telescope. The L-R method of deconvolution is efficient in resolving compact sources in crowded regions while simultaneously conserving their respective flux densities. We have analyzed itsmore » performance and convergence extensively through simulations and cross-correlations of the deconvolved images with available high-resolution maps. We present new science results from two BLAST surveys, in the Galactic regions K3-50 and IC 5146, further demonstrating the benefits of performing this deconvolution. We have resolved three clumps within a radius of 4.'5 inside the star-forming molecular cloud containing K3-50. Combining the well-resolved dust emission map with available multi-wavelength data, we have constrained the spectral energy distributions (SEDs) of five clumps to obtain masses (M), bolometric luminosities (L), and dust temperatures (T). The L-M diagram has been used as a diagnostic tool to estimate the evolutionary stages of the clumps. There are close relationships between dust continuum emission and both 21 cm radio continuum and {sup 12}CO molecular line emission. The restored extended large-scale structures in the Northern Streamer of IC 5146 have a strong spatial correlation with both SCUBA and high-resolution extinction images. A dust temperature of 12 K has been obtained for the central filament. We report physical properties of ten compact sources, including six associated protostars, by fitting SEDs to multi-wavelength data. All of these compact sources are still quite cold (typical temperature below {approx} 16 K) and are above the critical Bonner-Ebert mass. They have associated low-power young stellar objects. Further evidence for starless clumps has also been found in the IC 5146 region.« less

Deconvolution of Images from BLAST 2005: Insight into the K3-50 and IC 5146 Star-forming Regions

NASA Astrophysics Data System (ADS)

Roy, Arabindo; Ade, Peter A. R.; Bock, James J.; Brunt, Christopher M.; Chapin, Edward L.; Devlin, Mark J.; Dicker, Simon R.; France, Kevin; Gibb, Andrew G.; Griffin, Matthew; Gundersen, Joshua O.; Halpern, Mark; Hargrave, Peter C.; Hughes, David H.; Klein, Jeff; Marsden, Gaelen; Martin, Peter G.; Mauskopf, Philip; Netterfield, Calvin B.; Olmi, Luca; Patanchon, Guillaume; Rex, Marie; Scott, Douglas; Semisch, Christopher; Truch, Matthew D. P.; Tucker, Carole; Tucker, Gregory S.; Viero, Marco P.; Wiebe, Donald V.

2011-04-01

We present an implementation of the iterative flux-conserving Lucy-Richardson (L-R) deconvolution method of image restoration for maps produced by the Balloon-borne Large Aperture Submillimeter Telescope (BLAST). Compared to the direct Fourier transform method of deconvolution, the L-R operation restores images with better-controlled background noise and increases source detectability. Intermediate iterated images are useful for studying extended diffuse structures, while the later iterations truly enhance point sources to near the designed diffraction limit of the telescope. The L-R method of deconvolution is efficient in resolving compact sources in crowded regions while simultaneously conserving their respective flux densities. We have analyzed its performance and convergence extensively through simulations and cross-correlations of the deconvolved images with available high-resolution maps. We present new science results from two BLAST surveys, in the Galactic regions K3-50 and IC 5146, further demonstrating the benefits of performing this deconvolution. We have resolved three clumps within a radius of 4farcm5 inside the star-forming molecular cloud containing K3-50. Combining the well-resolved dust emission map with available multi-wavelength data, we have constrained the spectral energy distributions (SEDs) of five clumps to obtain masses (M), bolometric luminosities (L), and dust temperatures (T). The L-M diagram has been used as a diagnostic tool to estimate the evolutionary stages of the clumps. There are close relationships between dust continuum emission and both 21 cm radio continuum and 12CO molecular line emission. The restored extended large-scale structures in the Northern Streamer of IC 5146 have a strong spatial correlation with both SCUBA and high-resolution extinction images. A dust temperature of 12 K has been obtained for the central filament. We report physical properties of ten compact sources, including six associated protostars, by fitting SEDs to multi-wavelength data. All of these compact sources are still quite cold (typical temperature below ~ 16 K) and are above the critical Bonner-Ebert mass. They have associated low-power young stellar objects. Further evidence for starless clumps has also been found in the IC 5146 region.

Seasonal radiogenic isotopic variability of the African dust outflow to the tropical Atlantic Ocean and across to the Caribbean

NASA Astrophysics Data System (ADS)

Kumar, Ashwini; Abouchami, W.; Galer, S. J. G.; Singh, Satinder Pal; Fomba, K. W.; Prospero, J. M.; Andreae, M. O.

2018-04-01

In order to assess the impact of mineral dust on climate and biogeochemistry, it is paramount to identify the sources of dust emission. In this regard, radiogenic isotopes have recently been used successfully for tracing North African dust provenance and its transport across the tropical Atlantic to the Caribbean. Here we present two time series of radiogenic isotopes (Pb, Sr and Nd) in dusts collected at the Cape Verde Islands and Barbados in order to determine the origin of the dust and examine the seasonality of westerly dust outflow from Northern Africa. Aerosol samples were collected daily during two campaigns - February 2012 (winter) and June-July 2013 (summer) - at the Cape Verde Atmospheric Observatory (CVAO) on the island of São Vicente (16.9°N, 24.9°W). A one-year-long time series of aerosols from Barbados (13.16°N, 59.43°W) - a receptor region in the Caribbean - was sampled at a lower, monthly resolution. Our results resolve a seasonal isotopic signal at Cape Verde shown by daily variations, with a larger radiogenic isotope variability in winter compared to that in summer. This summer signature is also observed over Barbados, indicating similar dust provenance at both locations, despite different sampling years. This constrains the isotope fingerprint of Saharan Air Layer (SAL) dust that is well-mixed during its transport. This result provides unequivocal evidence for a permanent, albeit of variable strength, long-range transport of African dust to the Caribbean and is in full agreement with atmospheric models of North African dust emission and transport across the tropical Atlantic in the SAL. The seasonal isotopic variability is related to changes in the dust source areas - mainly the Sahara and Sahel regions - that are active all-year-round, albeit with variable contributions in summer versus the winter months. Our results provide little support for much dust contributed from the Bodélé Depression in Chad - the "dustiest" place on Earth - reaching Cape Verde and Barbados during the summer, while contributions during the winter months are likely patchy and minor at most. Importantly, a short-term isotopic excursion is resolved in the Cape Verde winter record during a dust outbreak on 06-08 February 2012. This features a highly radiogenic Pb and Sr and unradiogenic Nd signature, marking a clear shift in dust provenance relative to that of normal days. As the dust storm waned, continuous gradual changes are observed, reflecting mixing and progressive dilution with dust typical of normal days. These inferences from radiogenic isotope tracers are corroborated by both satellite images (CALIPSO and MODIS) and back-trajectory analyses. The radiogenic isotope fingerprinting of these presently-active North African dust sources, and especially the Saharan Air Layer, will prove invaluable in studies of past dust emission from Northern Africa, where imagery and back trajectory analysis are unavailable.

Source appointment of fine particle number and volume concentration during severe haze pollution in Beijing in January 2013.

PubMed

Liu, Zirui; Wang, Yuesi; Hu, Bo; Ji, Dongsheng; Zhang, Junke; Wu, Fangkun; Wan, Xin; Wang, Yonghong

2016-04-01

Extreme haze episodes repeatedly shrouded Beijing during the winter of 2012-2013, causing major environmental and health problems. To better understand these extreme events, particle number size distribution (PNSD) and particle chemical composition (PCC) data collected in an intensive winter campaign in an urban site of Beijing were used to investigate the sources of ambient fine particles. Positive matrix factorization (PMF) analysis resolved a total of eight factors: two traffic factors, combustion factors, secondary aerosol, two accumulation mode aerosol factors, road dust, and long-range transported (LRT) dust. Traffic emissions (54%) and combustion aerosol (27%) were found to be the most important sources for particle number concentration, whereas combustion aerosol (33%) and accumulation mode aerosol (37%) dominated particle volume concentrations. Chemical compositions and sources of fine particles changed dynamically in the haze episodes. An enhanced role of secondary inorganic species was observed in the formation of haze pollution. Regional transport played an important role for high particles, contribution of which was on average up to 24-49% during the haze episodes. Secondary aerosols from urban background presented the largest contributions (45%) for the rapid increase of fine particles in the severest haze episode. In addition, the invasion of LRT dust aerosols further elevated the fine particles during the extreme haze episode. Our results showed a clear impact of regional transport on the local air pollution, suggesting the importance of regional-scale emission control measures in the local air quality management of Beijing.

Ecological Restoration Programs Induced Amelioration of the Dust Pollution in North China Plain

NASA Astrophysics Data System (ADS)

Long, X.; Tie, X.; Li, G.; Junji, C.

2017-12-01

With Moderate Resolution Imaging Spectroradiometer (MODIS) land cover product (MCD12Q1), we quantitatively evaluate the ecological restoration programs (ERP) induced land cover change in China by calculating gridded the land use fraction (LUF). We clearly capture two obvious vegetation (grass and forest) protective barriers arise between the dust source region DSR and North China Plain NCP from 2011 to 2013. The WRF-DUST model is applied to investigate the impact of ERPs on dust pollution from 2 to 8 March 2016, corresponding to a national dust storm event over China. Despite some model biases, the WRF-DUST model reasonably reproduced the temporal variations of dust storm event, involving IOA of 0.96 and NMB of 2% for DSR, with IOA of 0.83 and NMB of -15% for downwind area of NCP. Generally, the WRF-DUST model well capture the spatial variations and evolutions of dust storm events with episode-average [PMC] correlation coefficient (R) of 0.77, especially the dust storm outbreak and transport evolution, involving daily average [PMC] R of 0.9 and 0.73 on 4-5 March, respectively. It is found that the ERPs generally reduce the dust pollution in NCP, especially for BTH, involving upper dust pollution control benefits of -15.3% (-21.0 μg m-3) for BTH, and -6.2% (-9.3 μg m-3) for NCP. We are the first to conduct model sensitivity studies to quantitatively evaluate the impacts of the ERPs on the dust pollution in NCP. And our narrative is independently based on first-hand sources, whereas government statistics.

A method of evaluating effects of antecedent precipitation on duststorms and its application to Yuma, Arizona, 1981-1988

USGS Publications Warehouse

MacKinnon, D.J.; Elder, D.F.; Helm, P.J.; Tuesink, M.F.; Nist, C.A.

1990-01-01

Precipitation causes several short- and long-term effects on wind-induced surface erodibility and subsequent dust emission. Among the principal effects considered by this paper are soil moisture, soil crusts, and vegetation. A quantitative method is developed to assess these effects using differences between the potential and the actual amounts of dust emitted from dust sources as inferred from surface meteorological measurements obtained downwind from those sources. The results of this assessment must be interpreted with caution, however, when the size and location of dust sources are unknown. Using meteorological data recorded near Yuma, Arizona at the Yuma Marine Corps Air Station (YMCAS), the method is applied to calculate the potential and actual amounts of dust emitted from upwind dust sources during the spring and fall/winter seasons between January 1, 1981 and May 31, 1988. (Spring is considered to be the period between February 1 and May 31; fall/winter, between October 1 and January 31.) Because summer precipitation is intermittent and wind patterns are localized, summer meteorological data are not used to evaluate regional correlations between precipitation and dust storms. For the period between 1981 and 1988, a correlation of -0.60 was found between fall/winter precipitation and the actual amount of dust emitted from sources upwind of YMCAS during the following spring. A particularly strong reduction in dust emission was noted during the springs of 1983 and 1984 following the start of an 'El Nino event' in fall/winter 1982. Photographs taken at a geological and meteorological data-collection (Geomet) site, located in the natural desert 25 km southeast of YMCAS, show a correspondence between increased antecedent precipitation recorded at the site and increased vegetation. Whereas the annual precipitation totals at YMCAS and the Geomet site from the beginning of 1982 through 1984 are high, their seasonal totals, especially during the fall/winter seasons, are disparate. This fall/winter precipitation disparity may account for evidence suggesting that significant vegetation growth occurred at dust sources upwind of YMCAS by spring 1983, but that such growth did not occur at the Geomet site until fall/ winter of 1983. Spatial inhomogeneity in fall/winter precipitation probably contributed to the relatively low correlation (-0.60) between fall/winter precipitation recorded at YMCAS and the actual amount of dust emitted from upwind sources during the following spring. ?? 1990 Kluwer Academic Publishers.

An integrated approach to assess heavy metal source apportionment in peri-urban agricultural soils.

PubMed

Huang, Ying; Li, Tingqiang; Wu, Chengxian; He, Zhenli; Japenga, Jan; Deng, Meihua; Yang, Xiaoe

2015-12-15

Three techniques (Isotope Ratio Analysis, GIS mapping, and Multivariate Statistical Analysis) were integrated to assess heavy metal pollution and source apportionment in peri-urban agricultural soils. The soils in the study area were moderately polluted with cadmium (Cd) and mercury (Hg), lightly polluted with lead (Pb), and chromium (Cr). GIS Mapping suggested Cd pollution originates from point sources, whereas Hg, Pb, Cr could be traced back to both point and non-point sources. Principal component analysis (PCA) indicated aluminum (Al), manganese (Mn), nickel (Ni) were mainly inherited from natural sources, while Hg, Pb, and Cd were associated with two different kinds of anthropogenic sources. Cluster analysis (CA) further identified fertilizers, waste water, industrial solid wastes, road dust, and atmospheric deposition as potential sources. Based on isotope ratio analysis (IRA) organic fertilizers and road dusts accounted for 74-100% and 0-24% of the total Hg input, while road dusts and solid wastes contributed for 0-80% and 19-100% of the Pb input. This study provides a reliable approach for heavy metal source apportionment in this particular peri-urban area, with a clear potential for future application in other regions. Copyright © 2015 Elsevier B.V. All rights reserved.

Gathering dust: A galaxy-wide study of dust emission from cloud complexes in NGC 300

NASA Astrophysics Data System (ADS)

Riener, M.; Faesi, C. M.; Forbrich, J.; Lada, C. J.

2018-05-01

Aims: We use multi-band observations by the Herschel Space Observatory to study the dust emission properties of the nearby spiral galaxy NGC 300. We compile a first catalogue of the population of giant dust clouds (GDCs) in NGC 300, including temperature and mass estimates, and give an estimate of the total dust mass of the galaxy. Methods: We carried out source detection with the multiwavelength source extraction algorithm getsources. We calculated physical properties, including mass and temperature, of the GDCs from five-band Herschel PACS and SPIRE observations from 100 to 500 μm; the final size and mass estimates are based on the observations at 250 μm that have an effective spatial resolution of 170 pc. We correlated our final catalogue of GDCs to pre-existing catalogues of HII regions to infer the number of GDCs associated with high-mass star formation and determined the Hα emission of the GDCs. Results: Our final catalogue of GDCs includes 146 sources, 90 of which are associated with known HII regions. We find that the dust masses of the GDCs are completely dominated by the cold dust component and range from 1.1 × 103 to 1.4 × 104 M⊙. The GDCs have effective temperatures of 13-23 K and show a distinct cold dust effective temperature gradient from the centre towards the outer parts of the stellar disk. We find that the population of GDCs in our catalogue constitutes 16% of the total dust mass of NGC 300, which we estimate to be about 5.4 × 106 M⊙. At least about 87% of our GDCs have a high enough average dust mass surface density to provide sufficient shielding to harbour molecular clouds. We compare our results to previous pointed molecular gas observations in NGC 300 and results from other nearby galaxies and also conclude that it is very likely that most of our GDCs are associated with complexes of giant molecular clouds. The catalogue is only available at the CDS via anonymous ftp to cdsarc.u-strasbg.fr (130.79.128.5) or via http://cdsarc.u-strasbg.fr/viz-bin/qcat?J/A+A/612/A81Herschel is an ESA space observatory with science instruments provided by European-led Principal Investigator consortia and with important participation from NASA.

Differences in ice nucleation behavior of arable and desert soil dust in deposition nucleation regime

NASA Astrophysics Data System (ADS)

Ullrich, Romy; Vogel, Franziska; Möhler, Ottmar; Höhler, Kristina; Schiebel, Thea

2017-04-01

Soil dust from arid and semi-arid regions is one of the most abundant aerosol types in the atmosphere with emission rates of about 1600 Tg per year (Andreae et al. (2009)). Therewith, soil dust plays an important role for the atmospheric radiative transfer and also for the formation of clouds. Soil dust refers to dust sampled from agricultural used areas, to dust from bare soil as well as to dust from desert regions. By mass-spectrometric measurements of the chemical composition of ice residuals, mineral dust as component of soil dust was found to be the major heterogeneous ice nucleating particle (INP) type (e.g. Cziczo et al. (2013)), in particular in the upper troposphere. Also in laboratory studies the ice nucleation efficiency of the different soil dusts was investigated. It was shown that desert dusts (Ullrich et al. (2017)) as well as soil dusts from arable regions (O'Sullivan et al. (2014), Tobo et al. (2014)) are efficient INP. However, there is still a lack of data for ice nucleation on soil dusts for temperatures below about 220 K. With the AIDA (Aerosol Interactions and Dynamics in the Atmosphere) cloud chamber, we are able to characterize the ice nucleation efficiency for different aerosol types to temperatures down to 180 K and high ice supersaturations. In order to extend the already existing AIDA data base for deposition nucleation on desert dusts and agricultural soil dusts, new experiments were done in the upper tropospheric temperature regime. This contribution will show the results of the new experiments with desert dust in comparison to existing data for higher temperatures. The first data analysis confirms the temperature dependent trend of the ice nucleation activity as discussed and parameterized in a recent paper by Ullrich et al. (2017). Furthermore, the update and extension of the recently published parameterization of deposition nucleation for desert dust to lower temperatures will be discussed. The experiments with agricultural soil dust will be compared to existing AIDA experiments at higher temperatures published by Steinke et al. (2016). Finally, the ice nucleation activity of both desert dust and agricultural soil dust will be compared for the upper tropospheric temperature regime. Andreae et al. (2009), Sources and Nature of Atmospheric Aerosols, in Aerosol Pollution Impact on Precipitation - A Scientific Review, Ch.3, Springer Netherlands, 45-89 Cziczo et al. (2013), Clarifying the Dominant Sources and Mechanisms of Cirrus Cloud Formation, Science, 340, 1320-1324 O'Sullivan et al. (2014), Ice nucleation by fertile soil dusts: relative importance of mineral and biogenic components, Atmos. Chem. Phys., 14, 1853-1867 Steinke et al. (2016), Ice nucleation activity of agricultural soil dust aerosols from Mongolia, Argentina and Germany, J. Geophys. Res., 121 Tobo et al. (2014), Organic matter matters for ice nuclei of agricultural soil origin, Atmos. Chem. Phys., 14, 8521-8531 Ullrich et al. (2017), A new ice nucleation active site parametrization for desert dust and soot, J. Atmos. Sci., in press

Tracking dust deposition around the North Pacific Gyre over the past 500kyr

NASA Astrophysics Data System (ADS)

Costa, K.; McManus, J. F.; Winckler, G.; Anderson, R. F.; Middleton, J. L.; Mukhopadhyay, S.

2017-12-01

Across the North Pacific, dust delivery and distribution depends on atmospheric transport and precipitation, and dust fluxes generally decrease with distance away from the Asian continent. While it is well established that dust fluxes vary on glacial-interglacial timescales, how the dust distribution from the source to the sediment may have evolved is poorly constrained, largely due to a lack of long dust flux records from this region. Here we reconstruct dust flux variability from six piston cores on the Juan de Fuca Ridge in the Northeastern Pacific over the past 500kyr using 232Th as a lithogenic tracer and 230Th normalization to calculate fluxes. Minimal spatial variability between the six cores allows the compilation of a single regional dust flux stack. Dust fluxes vary by a factor of two between glacial, high-dust flux, and interglacial, low-dust flux periods, consistent with global patterns. Interglacial periods MIS7 and MIS9 dust fluxes remain relatively high compared to the adjacent glacial periods MIS6 and MIS 8 so that dust fluxes are fairly constant (3.3±0.6 ug 232Th/cm2kyr) from 135-335ka, excepting the high-lithogenic feature at 272ka (turbidite). Dust fluxes may be highest in MIS10 (6.0 ug 232Th/cm2kyr) than more recent glacial periods, for example MIS2 (3.9 ug 232Th/cm2kyr). Five multicores add high-resolution data for the last 30kyr. We compare these new records from the Northeast Pacific with dust flux records from the Northwest Pacific and the Equatorial Pacific to better constrain how dust deposition varied at different locations around the North Pacific Gyre on glacial-interglacial timescales.

Extreme dust storm over the eastern Mediterranean in September 2015: satellite, lidar, and surface observations in the Cyprus region

NASA Astrophysics Data System (ADS)

Mamouri, Rodanthi-Elisavet; Ansmann, Albert; Nisantzi, Argyro; Solomos, Stavros; Kallos, George; Hadjimitsis, Diofantos G.

2016-11-01

A record-breaking dust storm originating from desert regions in northern Syria and Iraq occurred over the eastern Mediterranean in September 2015. In this contribution of a series of two articles (part 1, observations; part 2, atmospheric modeling), we provide a comprehensive overview of the aerosol conditions during this extreme dust outbreak in the Cyprus region. These observations are based on satellite observations (MODIS, moderate resolution imaging spectroradiometer) of aerosol optical thickness (AOT) and Ångström exponent, surface particle mass (PM10) concentrations measured at four sites in Cyprus, visibility observations at three airports in southern Cyprus and corresponding conversion products (particle extinction coefficient, dust mass concentrations), EARLINET (European Aerosol Research Lidar Network) lidar observations of dust vertical layering over Limassol, particle optical properties (backscatter, extinction, lidar ratio, linear depolarization ratio), and derived profiles of dust mass concentrations. Maximum 550 nm AOT exceeded values of 5.0, according to MODIS, and the mass loads were correspondingly > 10 g m-2 over Larnaca and Limassol during the passage of an extremely dense dust front on 8 September 2015. Hourly mean PM10 values were close to 8000 µg m-3 and the observed meteorological optical range (visibility) was reduced to 300-750 m at Larnaca and Limassol. The visibility observations suggest peak values of the near-surface total suspended particle (TSP) extinction coefficients of 6000 Mm-1 and thus TSP mass concentrations of 10 000 µg m-3. The Raman polarization lidar observations mainly indicated a double layer structure of the dust plumes (reaching to about 4 km height), pointing to at least two different dust source regions. Dust particle extinction coefficients (532 nm) already exceeded 1000 Mm-1 and the mass concentrations reached 2000 µg m-3 in the elevated dust layers on 7 September, more than 12 h before the peak dust front on 8 September reached the Limassol lidar station around local noon. Typical Middle Eastern dust lidar ratios around 40 sr were observed in the dense dust plumes. The particle depolarization ratio decreased from around 0.3 in the lofted dense dust layers to 0.2 at the end of the dust period (11 September), indicating an increasing impact of anthropogenic haze.

Using Nd and Sr isotopes to trace dust and volcanic inputs to soils on French Guadeloupe Island

NASA Astrophysics Data System (ADS)

Guo, J.; Pereyra, Y.; Ma, L.; Gaillardet, J.; Sak, P. B.; Bouchez, J.

2017-12-01

Soil is at the central part of the Critical Zone for its important roles in sustaining ecosystems and agriculture. At French Guadeloupe, a tropical humid volcanic island, previous studies have shown that the mineral nutrient elements such as K, Na, Ca, and Mg are highly depleted in the surface soil. And mineral nutrients introduced by dusts are an important mineral nutrient source for vegetation growth in this area. It is important to understand and quantify the sources of the mineral dust added to surface soils. Nd isotope ratios, due to their distinct signatures between two unique end-members in soils for this area: the young volcanic areas like Guadeloupe and the dust source region from the old continental shields like Sahara Desert, can be a robust tracer to understand this critical process. Nevertheless, Sr isotope ratios can trace the inputs of marine aerosols. Here we present a new Nd isotope study on Guadeloupe soil depth profiles, combined with previous Sr isotope data, to fingerprint the sources of dust and volcanic inputs into soils. Soil samples from three surface profiles (0 - 1000cm deep) at different locations of the Guadeloupe Island were systematically analyzed. The results show distinct depth variations for Nd isotope signature along profiles. For all profiles, deep soils are relatively consisted with bedrock value (ɛNd: 5.05). But in surface soils (0-600cm), unlike Sr isotope ratios that are significantly modified by marine aerosol input, Nd isotope ratios show similar decrease (to ɛNd:-10) and frequent fluctuations toward the surface, suggesting dust is the dominant source of Nd in these soils. This conclusion is further supported by REE and other trace element data. Thus, with a simplified two end-member model, Sahara dust contributes the Nd percentages in soils varying from 10.7% at the deepest profiles to 69.5% on surface, showing a significant amount of Nd on the surface soil came from dust source. The deep soil profiles are also characterized by the presence of Nd isotope spikes with negative values, suggesting dust signatures at depth. Such a feature could be related to the presence of a paleo-soil surface at the spike depth that was buried by later volcanic eruption. Both Nd and Sr isotopes hence show dust and volcanic inputs are important factors for soil developments on French Guadeloupe Island.

Risk of Adverse Health and Performance Effects of Celestial Dust Exposure

NASA Technical Reports Server (NTRS)

Scully, Robert R.; Meyers, Valerie E.

2015-01-01

Crew members can be directly exposed to celestial dust in several ways. After crew members perform extravehicular activities (EVAs), they may introduce into the habitat dust that will have collected on spacesuits and boots. Cleaning of the suits between EVAs and changing of the Environmental Control Life Support System filters are other operations that could result in direct exposure to celestial dusts. In addition, if the spacesuits used in exploration missions abrade the skin, as current EVA suits have, then contact with these wounds would provide a source of exposure. Further, if celestial dusts gain access to a suit's interior, as was the case during the Apollo missions, the dust could serve as an additional source of abrasions or enhance suit-induced injuries. When a crew leaves the surface of a celestial body and returns to microgravity, the dust that is introduced into the return vehicle will "float," thus increasing the opportunity for ocular and respiratory injury. Because the features of the respirable fraction of lunar dusts indicate they could be toxic to humans, NASA conducted several studies utilizing lunar dust simulants and authentic lunar dust to determine the unique properties of lunar dust that affect physiology, assess the dermal and ocular irritancy of the dust, and establish a permissible exposure limit for episodic exposure to airborne lunar dust during missions that would involve no more than 6 months stay on the lunar surface. Studies, with authentic lunar soils from both highland (Apollo 16) and mare (Apollo17) regions demonstrated that the lunar soil is highly abrasive to a high fidelity model of human skin. Studies of lunar dust returned during the Apollo 14 mission from an area of the moon in which the soils were comprised of mineral constituents from both major geological regions (highlands and mares regions) demonstrated only minimal ocular irritancy, and pulmonary toxicity that was less than the highly toxic terrestrial crystalline silica (Permissible Exposure Limit [PEL] 0.05 mg/m3) but more toxic than the nuisance dust titanium dioxide (TiO2 [PEL 5.0 mg/m3]). A PEL for episodic exposure to airborne lunar dust during a six-month stay on the lunar surface was established, in consultation with an independent, extramural panel of expert pulmonary toxicologists, at 0.3 mg/m3. The PEL provided for lunar dust is limited to the conditions and exposure specified therefore additional research remains to be accomplished with lunar dust to further address the issues of activation, address other areas of more unique lunar geology (Glotch et al., 2010; Greenhagen et al., 2010), examine potential toxicological effects of inhaled or ingested dust upon other organ systems, such cardiovascular, nervous systems, and examine effects of acute exposure to massive doses of dust such as may occur during off-nominal situations. Work to support the establishment of PELs for Martian dust and dusts of asteroids remains to be accomplished. The literature that describes health effects of exposure to toxic terrestrial dusts provides substantial basis for concern that prolonged exposure to respirable celestial dust could be detrimental to human health. Celestial bodies where a substantial portion of the dust is in the respirable range or where the dusts have large reactive surface areas or contain transition metals or volatile organics, represent greater risks of adverse effects from exposure to the dust. It is possible that in addition to adverse effects to the respiratory system, inhalation and ingestion of celestial dusts could pose risks to other systems

An Extensive Study on Dynamical aspects of Dust Storm over the United Arab Emirates during 18-20 March 2012

NASA Astrophysics Data System (ADS)

Basha, Ghouse; Phanikumar, Devulapalli V.; Ouarda, Taha B. M. J.

2015-04-01

On 18 March 2012, a super dust storm event occurred over Middle East (ME) and lasted for several hours. Following to this, another dust storm occurred on early morning of 20 March 2012 with almost higher intensity. Both these storms reduced the horizontal visibility to few hundreds of meters and represented as one of the most intense and long duration dust storms over United Arab Emirates (UAE) in recent times. These storms also reduced the air quality in most parts of the ME implying the shutdown of Airports, schools and hundreds of people were hospitalized with respirational problems. In the context of the above, we have made a detailed study on the dynamical processes leading to triggering of dust storm over UAE and neighboring regions. We have also analyzed its impact on surface, and vertical profiles of background parameters and aerosols during the dust storm period by using ground-based, space borne, dust forecasting model, and reanalysis data sets. The synoptic and dynamic conditions responsible for the occurrence of the dust storm are discussed extensively by using European Centre for Medium-Range Weather Forecasts (ECMWF) ERA interim reanalysis data sets. The Impact of dust storm on surface and upper air radiosonde measurements and aerosol optical properties are also investigated before, during and after the dust storm event. During the dust storm, surface temperature decreased by 15oC when compared to before and after the event. PM10 values significantly increased maximum of about 1600µg/m3. Spatial variation of Aerosol Optical Depth (AOD) from Moderate-resolution Imaging Spectroradiometer (MODIS) and Ozone Monitoring Instrument (OMI) aerosol index (AI) exhibited very high values during the event and source region can be identified of dust transport to our region with this figure. The total attenuated backscatter at 550nm from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite shows the vertical extent of dust up to 8km. The dynamics of this event is related to coupling of subtropical jet and polar jet over the Saudi Arabia region, which leads to massive dust storm generation and dust transport through Rub-Al-Khali, and Persian Gulf over the UAE region. AOD from ground based measurements showed fourfold increase from 0.2 to 1.8 during the event implying an atmospheric forcing of ~ 150 Wm-2. In addition, vertical profile of heating rate showed heating of ~1.5 K/day at 3-4 km during the event. In the view of the above, the present event is discussed in the light of current understanding of dust storm aerosol optical and physical processes and associated dynamics over UAE region.

WEAK AND COMPACT RADIO EMISSION IN EARLY HIGH-MASS STAR-FORMING REGIONS. I. VLA OBSERVATIONS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rosero, V.; Hofner, P.; Claussen, M.

2016-12-01

We present a high-sensitivity radio continuum survey at 6 and 1.3 cm using the Karl G. Jansky Very Large Array toward a sample of 58 high-mass star-forming regions. Our sample was chosen from dust clumps within infrared dark clouds with and without IR sources (CMC–IRs and CMCs, respectively), and hot molecular cores (HMCs), with no previous, or relatively weak radio continuum detection at the 1 mJy level. Due to the improvement in the continuum sensitivity of the Very Large Array, this survey achieved map rms levels of ∼3–10  μ Jy beam{sup −1} at sub-arcsecond angular resolution. We extracted 70 continuum sourcesmore » associated with 1.2 mm dust clumps. Most sources are weak, compact, and prime candidates for high-mass protostars. Detection rates of radio sources associated with the millimeter dust clumps for CMCs, CMC–IRs, and HMCs are 6%, 53%, and 100%, respectively. This result is consistent with increasing high-mass star formation activity from CMCs to HMCs. The radio sources located within HMCs and CMC–IRs occur close to the dust clump centers, with a median offset from it of 12,000 au and 4000 au, respectively. We calculated 5–25 GHz spectral indices using power-law fits and obtained a median value of 0.5 (i.e., flux increasing with frequency), suggestive of thermal emission from ionized jets. In this paper we describe the sample, observations, and detections. The analysis and discussion will be presented in Paper II.« less

Dust composition changes from Taylor Glacier (East Antarctica) during the last glacial-interglacial transition: A multi-proxy approach

NASA Astrophysics Data System (ADS)

Aarons, Sarah M.; Aciego, Sarah M.; Arendt, Carli A.; Blakowski, Molly A.; Steigmeyer, August; Gabrielli, Paolo; Sierra-Hernández, M. Roxana; Beaudon, Emilie; Delmonte, Barbara; Baccolo, Giovanni; May, Nathaniel W.; Pratt, Kerri A.

2017-04-01

Mineral dust is transported in the atmosphere and deposited in oceans, ice sheets and the terrestrial biosphere. Temporal changes in locations of dust source areas and transport pathways have implications for global climate and biogeochemical cycles. The chemical and physical characterization of the dust record preserved in ice cores is useful for identifying of dust source regions, dust transport, dominant wind direction and storm trajectories. Here, we present a 50,000-year geochemical characterization of mineral dust entrapped in a horizontal ice core from the Taylor Glacier in East Antarctica. Strontium (Sr) and neodymium (Nd) isotopes, grain size distribution, trace and rare earth element (REE) concentrations, and inorganic ion (Cl- and Na+) concentrations were measured in 38 samples, corresponding to a time interval from 46 kyr before present (BP) to present. The Sr and Nd isotope compositions of insoluble dust in the Taylor Glacier ice shows distinct changes between the Last Glacial Period (LGP in this study ranging from ∼46.7-15.3 kyr BP) the early Holocene (in this study ranging from ∼14.5-8.7 kyr BP), and zero-age samples. The 87Sr/86Sr isotopic composition of dust in the Taylor Glacier ice ranged from 0.708 to 0.711 during the LGP, while the variability during the early Holocene is higher ranging from 0.707 to 0.714. The εNd composition ranges from 0.1 to -3.9 during the LGP, and is more variable from 1.9 to -8.2 during the early Holocene. The increased isotopic variability during the early Holocene suggests a shift in dust provenance coinciding with the major climate transition from the LGP to the Holocene. The isotopic composition and multiple physical and chemical constraints support previous work attributing Southern South America (SSA) as the main dust source to East Antarctica during the LGP, and a combination of both local Ross Sea Sector dust sources and SSA after the transition into the Holocene. This study provides the first high time resolution data showing variations in dust provenance to East Antarctic ice during a major climate regime shift, and we provide evidence of changes in the atmospheric transport pathways of dust following the last deglaciation.

A quantitative evaluation of the 3-8 July 2009 Shamal dust storm

NASA Astrophysics Data System (ADS)

Hamidi, Mehdi; Kavianpour, Mohammad Reza; Shao, Yaping

2017-02-01

In this paper, a quantitative evaluation of the severe dust storm which occurred in the Middle East during 3-8 July 2009 is presented. The quantification is based on the numerical simulation using the WRF/Chem-D model which has been verified and calibrated for the Middle East region. It is found that, during the 3-8 July 2009 event, more than 9.67 Tg dust were emitted from the study area and the maximum simulated dust emission rate is 540 (μg m-2 s-1). The west of Iraq, east of Syria and northwest of Jordan (Al-Nafud desert and western Euphrates alluvial plain) are found to be the most active areas of dust emission, contributing much to the dust emission from the Middle East region. In this study, more that 60% of dust particles were emitted from these areas and less than 10% were emitted from Iran dust sources. About 21% of the deposited dust was deposited in Iran land, while 79% in other parts of the study area. The dust load in the study area was estimated to be more than 0.3 g m-2. The residence time of dust in the atmosphere was 6.2 days over the study area, 7.8 days over Iran and 6 days over other parts. The simulation results exhibit that Iran contribution in emission rate in the study area is much lower than its contribution in dust deposition and residence time and the conclusion of this study can demonstrate the necessity of forming cooperation for suppressing the severe dust events.

The effects of interplanetary dust impacts on the accumulation of volatiles in the lunar permanently shadowed regions

NASA Astrophysics Data System (ADS)

Horanyi, Mihaly; Szalay, Jamey

2017-10-01

The lunar regolith has been formed, and remains continually reworked, by the intermitten impacts of comets, asteroids, meteoroids, and the continual bombardment by interplanetary dust particles (IDP). Thick atmospheres protect Venus, Earth, and Mars, ablating the incoming IDPs into “shooting stars” that rarely reach the surface. However, the surfaces of airless bodies near 1 AU are directly exposed to the high-speed (>> 1 km/s) IDP impacts. The Moon is expected to be bombarded by 5x103 kg/day of IDPs arriving with a characteristic speed of ~ 20 km/s. The IDP sources impacting the Moon at high latitudes remain largely uncharacterized due to the lack of optical and radar observations in the polar regions on Earth. These high latitude sources have very large impact speeds in the range of 30 < v < 50 km/ hence they are expected to have a significant effect on the lunar surface, including the removal and burial of volatile deposits in the lunar polar regions.Water is thought to be continually delivered to the Moon through geological timescales by water-bearing comets and asteroids, and produced continuously in situ by the impacts of solar wind protons of oxygen rich minerals exposed on the surface. IDPs are an unlikely source of water due to their long UV exposure in the inner solar system, but their high-speed impacts can mobilize secondary ejecta dust particles, atoms and molecules, some with high-enough speed to escape the Moon. Other surface processes that can lead to mobilization, transport and loss of water molecules and other volatiles include solar heating, photochemical processes, and solar wind sputtering. Since none of these are at work in permanently shadowed regions (PSR), dust impacts remain the dominant process to dictate the evolution of volatiles in PSRs. The competing effects of dust impacts are: a) ejecta production leading to loss out of a PSR; b) gardening and overturning the regolith; and c) the possible accumulation of impact ejecta, leading to the burial of the volatiles. This talk will summarize the expected effects of dust impacts on volatile accumulation in the lunar PSRs based on theoretical models, recent laboratory results, and observations by the LADEE spacecraft.

Revisiting the Observed Correlation Between Weekly Averaged Indian Monsoon Precipitation and Arabian Sea Aerosol Optical Depth

NASA Astrophysics Data System (ADS)

Sharma, D.; Miller, R. L.

2017-12-01

Dust influences the Indian summer monsoon on seasonal timescales by perturbing atmospheric radiation. On weekly time scales, aerosol optical depth retrieved by satellite over the Arabian Sea is correlated with Indian monsoon precipitation. This has been interpreted to show the effect of dust radiative heating on Indian rainfall on synoptic (few-day) time scales. However, this correlation is reproduced by Earth System Model simulations, where dust is present but its radiative effect is omitted. Analysis of daily variability suggests that the correlation results from the effect of precipitation on dust through the associated cyclonic circulation. Boundary layer winds that deliver moisture to India are responsible for dust outbreaks in source regions far upwind, including the Arabian Peninsula. This suggests that synoptic variations in monsoon precipitation over India enhance dust emission and transport to the Arabian Sea. The effect of dust radiative heating upon synoptic monsoon variations remains to be determined.

Revisiting the observed correlation between weekly averaged Indian monsoon precipitation and Arabian Sea aerosol optical depth

NASA Astrophysics Data System (ADS)

Sharma, Disha; Miller, Ron L.

2017-10-01

Dust influences the Indian summer monsoon on seasonal time scales by perturbing atmospheric radiation. On weekly time scales, aerosol optical depth retrieved by satellite over the Arabian Sea is correlated with Indian monsoon precipitation. This has been interpreted to show the effect of dust radiative heating on Indian rainfall on synoptic (few-day) time scales. However, this correlation is reproduced by Earth System Model simulations, where dust is present but its radiative effect is omitted. Analysis of daily variability suggests that the correlation results from the effect of precipitation on dust through the associated cyclonic circulation. Boundary layer winds that deliver moisture to India are responsible for dust outbreaks in source regions far upwind, including the Arabian Peninsula. This suggests that synoptic variations in monsoon precipitation over India enhance dust emission and transport to the Arabian Sea. The effect of dust radiative heating upon synoptic monsoon variations remains to be determined.

Anthropogenic Air Pollution Observed Near Dust Source Regions in Northwestern China During Springtime 2008

NASA Technical Reports Server (NTRS)

Li, Can; Tsay, Si-Chee; Fu, Joshua S.; Dickerson, Russell R.; Ji, Qiang; Bell, Shaun W.; Gao, Yang; Zhang, Wu; Huang, Jianping; Li, Zhanqing;

Characteristics of Dust Deposition at High Elevation Sites in Caucasus Over the Past 190 years Recorded in Ice Cores.

NASA Astrophysics Data System (ADS)

Kutuzov, Stanislav; Ginot, Patrick; Mikhaenko, Vladimir; Krupskaya, Victoria; Legrand, Michel; Preunkert, Suzanne; Polukhov, Alexey; Khairedinova, Alexandra

2017-04-01

The nature and extent of both radiative and geochemical impacts of mineral dust on snow pack and glaciers depend on physical and chemical properties of dust particles and its deposition rates. Ice cores can provide information about amount of dust particles in the atmosphere and its characteristic and also give insights on strengths of the dust sources and its changes in the past. A series of shallow ice cores have been obtained in Caucasus mountains, Russia in 2004 - 2015. A 182 meter ice core has been recovered at the Western Plateau of Mt. Elbrus (5115 m a.s.l.) in 2009. The ice cores have been dated using stable isotopes, NH4+ and succinic acid data with the seasonal resolution. Samples were analysed for chemistry, concentrations of dust and black carbon, and particle size distributions. Dust mineralogy was assessed by XRD. Individual dust particles were analysed using SEM. Dust particle number concentration was measured using the Markus Klotz GmbH (Abakus) implemented into the CFA system. Abakus data were calibrated with Coulter Counter multisizer 4. Back trajectory cluster analysis was used to assess main dust source areas. It was shown that Caucasus region experiencing influx of mineral dust from the Sahara and deserts of the Middle East. Mineralogy of dust particles of desert origin was significantly different from the local debris material and contained large proportion of calcite and clay minerals (kaolinite, illite, palygorskite) associated with material of desert origin. Annual dust flux in the Caucasus Mountains was estimated as 300 µg/cm2 a-1. Particle size distribution depends on individual characteristics of dust deposition event and also on the elevation of the drilling site. The contribution of desert dust deposition was estimated as 35-40 % of the total dust flux. Average annual Ca2+ concentration over the period from 1824 to 2013 was of 150 ppb while some of the strong dust deposition events led to the Ca2+ concentrations reaching 4400 ppb. An increase of dust and Ca2+ concentration was registered since the beginning of XX century. The ice core record depicts also a prominent increase of dust concentration in 1980's which may be related to the increase of dust sources strength in North Africa.

The relationship between the Asian dust and Arctic Oscillation: An observational investigation

NASA Astrophysics Data System (ADS)

Lee, Y.; Kim, J.; Cho, H.

2009-12-01

The Arctic Oscillation (AO) represents the leading empirical orthogonal function of winter sea level pressure (SLP) fields, which resembles North Atlantic Oscillation, but has a more zonally symmetric structure (Thompson and Wallace, 1998; Wallace, 2000; Wu and Wang, 2002). This primary mode of the internal dynamics in the atmosphere predominates the Extratropical Northern Hemisphere circulation from surface to the lower stratosphere showing an equivalent barotropic structure during cold season(November-April) (Thompson and Wallace, 2000). Also, the Asian dust storms show strong interannual variation (Sun et al., 2001; Yoshino, 2002; Zhao et al., 2006; Hara et al., 2006), which are suggested to be associated with climate indices. Therefore, the purpose of this study is to identify the possible connection for the AO and the Asian dust emission during periods from late winter to spring, based on the observational investigations. In order to examine these complex associations closely, the Aerosol Index (AI) from Total Ozone Mapping Spectrometer (TOMS) are used starting from November 1978 to December 1999, except for data pause from May 1993 to August 1996. SLP and geopotential height at 500hPa (Z500) monthly fields are derived from the European Centre for Medium-Range Weather Forecasts (ECMWF) reanalyses (1958-2001). Also, source regions of Asian dust are mainly focused on three source areas, including the Taklimakan Desert (R1), Badain Jaran Desert (R2), and Mongolia (R3) in this study. In composite study during different phases of AO, the AO exhibits a “negative phase” with relatively high pressure over the polar region and low pressure at mid-latitudes (about 45 degrees North). In strong “negative phase” of AO, decrease of AO is found to be associated with decreases of local tropospheric temperature, U-wind, and geopotential height and strong north-south gradients over the source regions of Asian dust. Therefore, we also notice that a negative index phase in the spring AO results in the strengthened East Asian Trough at 500hPa and a significant pressure decrease in the lower atmosphere, which is favorable for producing the stronger Asian dust emission.

Source reconciliation of atmospheric dust causing visibility impairment in Class I areas of the western United States

NASA Astrophysics Data System (ADS)

Kavouras, Ilias G.; Etyemezian, Vicken; Dubois, David W.; Xu, Jin; Pitchford, Marc

2009-01-01

Aerosol data from the Interagency Monitoring of Protected Visual Environments (IMPROVE) network, air mass backward trajectories, land use maps, soil characteristics maps, diagnostic ratios of elemental composition, and multivariate linear regression were utilized as part of a semiquantitative analysis. The purpose of the analysis was to determine the types of dust-causing events that contribute to low visibility at a given site when the sum of extinction from coarse mass (CM) and fine soil (FS) was larger than any other aerosol component and the reconstructed aerosol extinction coefficient was among the 20% highest (calculated on a calendar year basis) for that site. For these "worst dust days," the above tools were used to ascribe the cause of low visibility to one of the following types of events: (1) transcontinental transport of dust originating from Asia; (2) windblown dust events from sources located nearby the site and; (3) transport of windblown dust from sources upwind of the site. Depending on the weight of evidence, a low or high level of confidence was associated with the assignment of one of these three events. Absence of convincing evidence resulted in ascribing the worst dust day to "undetermined events." Of the 610 worst dust days over the 2001-2003 period, 51% were associated with one of the three event types with high confidence and an additional 30% were accounted for with low confidence. Of the 496 worst dust days associated with an event (either low or high confidence), Asian dust was the assigned event on 55 days (for 2001-2002), locally generated windblown dust on 201 days, and transport from upwind source areas susceptible to wind erosion on 240 days. Events associated with windblown episodes from source areas in the United States and Mexico exhibited the highest dust concentrations. Asian dust events were associated with lower dust concentrations and a larger FS-to-CM ratio. Some variations between Asian dust and continental North American dust were observed in organic matter (OMC), black carbon (LAC), and nitrate (NO3-) content. None of the tools used in this study was adequate for identifying events associated with mechanically released dust by anthropogenic activities including, agriculture, construction and motor vehicle travel on paved and unpaved roads. Some of the worst dust days may have been caused by these types of activities, especially in central Arizona and northern and Southern California, where the fraction of undetermined events was higher than in other regions within the western United States. All in all, the methods and results of this study can help improve the performance of large-scale dust emission models and provide insight into the distribution of the types of events that cause dust resultant haze in relatively remote areas of the western United States.

Modeling and observations of dust aerosols during the North American Monsoon

NASA Astrophysics Data System (ADS)

Arellano, A. F.; Raman, A.; Brost, J.; Sorooshian, A.

2016-12-01

Intense dust storms during North American Monsoon (NAM) pose a significant threat to local/regional air quality, economy, and public health. Convection-driven storms (or haboobs) in Arizona and in the southwest US have been given far less attention compared to those in Africa and Middle East. Blowing dusts from these haboobs typically lasts for 3-6 hours and accumulate more than 1000 µg m-3 of PM10 in the atmosphere. However, it is not clear whether haboobs are increasing in intensity and/or frequency in Arizona. Here, we address two science questions: 1) Do haboobs impact the observed trends in aerosol abundance in the NAM region?, 2) What are our current capabilities and limitations in understanding, monitoring, and assessing haboobs and their impacts? For 1), we calculated the trends of enhancements in aerosol optical depth (AOD) from Terra MODIS over dust hotspots in the NAM alley and and surrounding region (dust cluster). Both show similar decreasing trends before the monsoon. However, during the monsoon, a decreasing trend in AOD is more prominent in the dust cluster than in NAM alley. We attribute this to an apparent modulation of dust in the NAM alley by haboobs. Despite increase in rainfall during this period, we infer that the increase in dust sources in the NAM alley obscures the decreasing AOD trend. For 2), we conducted simulations simulations of these haboobs using WRF-Chem with GOCART AFWA scheme at convective resolving scales ( 1 km). Our case study for the 5 July 2011 haboob indicate that the downbursts occurred near Tucson and generated diverging high intensity winds, resulting to cold pools propagating towards Phoenix. We find that WRF-Chem captures the timing of the haboob but severely underestimates the magnitude of dust concentrations that reached as high as 2000 µg m-3 at USEPA Phoenix stations. The impact of the haboob was seen as far as 350 km northwest of Phoenix at an altitude of 2-4 km on 6 July. We find two major limitations in our simulations: 1) lack of dynamic high resolution land cover for prescribing dust sources, and 2) lack of observing system capability especially high temporal resolution, remotely-sensed measurements for monitoring and assessment. Future geostationary missions together with synergistic use of current and future expansion of in-situ measurements can improve these limitations.

Understanding the Transport of Patagonian Dust and Its Influence on Marine Biological Activity in the South Atlantic Ocean

NASA Technical Reports Server (NTRS)

Johnson, Matthew; Meskhidze, Nicholas; Kiliyanpilakkil, Praju; Gasso, Santiago

2010-01-01

Modeling and remote sensing techniques were applied to examine the horizontal and vertical transport pathways of Patagonian dust and quantify the effect of soluble-iron- laden mineral dust deposition on marine primary productivity in the South Atlantic Ocean (SAO) surface waters. The global chemistry transport model GEOS-Chem, implemented with an iron dissolution scheme, was applied to evaluate the atmospheric transport and deposition of mineral dust and bioavailable iron during two dust outbreaks originating in the source regions of Patagonia. In addition to this "rapidly released" iron, offline calculations were also carried out to estimate the amount of bioavailable iron leached during the residence time of dust in the ocean mixed layer. Model simulations showed that the horizontal and vertical transport pathways of Patagonian dust plumes were largely influenced by the synoptic meteorological patterns of high and low pressure systems. Model-predicted horizontal and vertical transport pathways of Patagonian dust over the SAO were in reasonable agreement with remotely-sensed data. Comparison between remotely-sensed and offline calculated ocean surface chlorophyll-a concentrations indicated that, for the two dust outbreaks examined in this study, the deposition of bioavailable iron in the SAO through atmospheric pathways was insignificant. As the two dust transport episodes examined here represent typical outflows of mineral dust from South American sources, our study suggests that the atmospheric deposition of mineral dust is unlikely to induce large scale marine primary productivity and carbon sequestration in the South Atlantic sector of the Southern Ocean.

Comparison of Key Absorption and Optical Properties Between Pure and Transported Anthropogenic Dust over East and Central Asia

NASA Technical Reports Server (NTRS)

Bi, Jianrong; Huang, Jianping; Holben, Brent N.; Zhang, Guolong

2016-01-01

Asian dust particulate is one of the primary aerosol constituents in the Earth-atmosphere system that exerts profound influences on environmental quality, human health, the marine biogeochemical cycle, and Earth's climate. To date, the absorptive capacity of dust aerosol generated from the Asian desert region is still an open question. In this article, we compile columnar key absorption and optical properties of mineral dust over East and Central Asian areas by utilizing the multiyear quality-assured datasets observed at 13 sites of the Aerosol Robotic Network (AERONET). We identify two types of Asian dust according to threshold criteria from previously published literature. (1) The particles with high aerosol optical depth at 440 nm (AOD(440) > or = 0.4) and a low Angstrom wavelength exponent at 440-870 nm (alpha < 0.2) are defined as Pure Dust (PDU), which decreases disturbance of other non-dust aerosols and keeps high accuracy of pure Asian dust. (2) The particles with AOD(440) > or = 0.4 and 0.2 < alpha < 0.6 are designated as Transported Anthropogenic Dust (TDU), which is mainly dominated by dust aerosol and might mix with other anthropogenic aerosol types. Our results reveal that the primary components of high AOD days are predominantly dust over East and Central Asian regions, even if their variations rely on different sources, distance from the source, emission mechanisms, and meteorological characteristics. The overall mean and standard deviation of single-scattering albedo, asymmetry factor, real part and imaginary part of complex refractive index at 550 nm for Asian PDU are 0.935 +/- 0.014, 0.742 +/- 0.008, 1.526 +/- 0.029, and 0.00226 +/- 0.00056, respectively, while corresponding values are 0.921 +/- 0.021, 0.723 +/- 0.009, 1.521 +/- 0.025, and 0.00364 +/- 0.0014 for Asian TDU. Aerosol shortwave direct radiative effects at the top of the atmosphere (TOA), at the surface (SFC), and in the atmospheric layer (ATM) for Asian PDU (alpha < 0.2) and TDU (0.2 < alpha < 0.6) computed in this study, are a factor of 2 smaller than the results of Optical Properties of Aerosols and Clouds (OPAC) mineral-accumulated (mineral-acc.) and mineral-transported (mineral-tran.) modes. Therefore, we are convinced that our results hold promise for updating and improving accuracies of Asian dust characteristics in present-day remote sensing applications and regional or global climate models.

Comparison of key absorption and optical properties between pure and transported anthropogenic dust over East and Central Asia

NASA Astrophysics Data System (ADS)

Bi, Jianrong; Huang, Jianping; Holben, Brent; Zhang, Guolong

2016-12-01

Asian dust particulate is one of the primary aerosol constituents in the Earth-atmosphere system that exerts profound influences on environmental quality, human health, the marine biogeochemical cycle, and Earth's climate. To date, the absorptive capacity of dust aerosol generated from the Asian desert region is still an open question. In this article, we compile columnar key absorption and optical properties of mineral dust over East and Central Asian areas by utilizing the multiyear quality-assured datasets observed at 13 sites of the Aerosol Robotic Network (AERONET). We identify two types of Asian dust according to threshold criteria from previously published literature. (1) The particles with high aerosol optical depth at 440 nm (AOD440 ≥ 0.4) and a low Ångström wavelength exponent at 440-870 nm (α < 0.2) are defined as Pure Dust (PDU), which decreases disturbance of other non-dust aerosols and keeps high accuracy of pure Asian dust. (2) The particles with AOD440 ≥ 0.4 and 0.2 < α < 0.6 are designated as Transported Anthropogenic Dust (TDU), which is mainly dominated by dust aerosol and might mix with other anthropogenic aerosol types. Our results reveal that the primary components of high AOD days are predominantly dust over East and Central Asian regions, even if their variations rely on different sources, distance from the source, emission mechanisms, and meteorological characteristics. The overall mean and standard deviation of single-scattering albedo, asymmetry factor, real part and imaginary part of complex refractive index at 550 nm for Asian PDU are 0.935 ± 0.014, 0.742 ± 0.008, 1.526 ± 0.029, and 0.00226 ± 0.00056, respectively, while corresponding values are 0.921 ± 0.021, 0.723 ± 0.009, 1.521 ± 0.025, and 0.00364 ± 0.0014 for Asian TDU. Aerosol shortwave direct radiative effects at the top of the atmosphere (TOA), at the surface (SFC), and in the atmospheric layer (ATM) for Asian PDU (α < 0.2) and TDU (0.2 < α < 0.6) computed in this study, are a factor of 2 smaller than the results of Optical Properties of Aerosols and Clouds (OPAC) mineral-accumulated (mineral-acc.) and mineral-transported (mineral-tran.) modes. Therefore, we are convinced that our results hold promise for updating and improving accuracies of Asian dust characteristics in present-day remote sensing applications and regional or global climate models.

Nearly a Decade of CALIPSO Observations of Asian and Saharan Dust Properties Near Source and Transport Regions

NASA Technical Reports Server (NTRS)

Omar, Ali H.; Liu, Z.; Tackett, J.; Vaughan, M.; Trepte, C.; Winker, D.; H. Yu,

2015-01-01

The lidar on the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission, makes robust measurements of dust and has generated a length of record that is significant both seasonally and inter-annually. We exploit this record to determine a multi-year climatology of the properties of Asian and Saharan dust, in particular seasonal optical depths, layer frequencies, and layer heights of dust gridded in accordance with the Level 3 data products protocol, between 2006-2015. The data are screened using standard CALIPSO quality assurance flags, cloud aerosol discrimination (CAD) scores, overlying features and layer properties. To evaluate the effects of transport on the morphology, vertical extent and size of the dust layers, we compare probability distribution functions of the layer integrated volume depolarization ratios, geometric depths and integrated attenuated color ratios near the source to the same distributions in the far field or transport region. CALIPSO is collaboration between NASA and Centre National D'études Spatiales (CNES), was launched in April 2006 to provide vertically resolved measurements of cloud and aerosol distributions. The primary instrument on the CALIPSO satellite is the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), a near-nadir viewing two-wavelength polarization-sensitive instrument. The unique nature of CALIOP measurements make it quite challenging to validate backscatter profiles, aerosol type, and cloud phase, all of which are used to retrieve extinction and optical depth. To evaluate the uncertainty in the lidar ratios, we compare the values computed from dust layers overlying opaque water clouds, considered nominal, with the constant lidar ratio value used in the CALIOP algorithms for dust. We also explore the effects of noise on the CALIOP retrievals at daytime by comparing the distributions of the properties at daytime to the nighttime distributions.

Advances in understanding mineral dust and boundary layer processes over the Sahara from Fennec aircraft observations

NASA Astrophysics Data System (ADS)

Ryder, C. L.; McQuaid, J. B.; Flamant, C.; Rosenberg, P. D.; Washington, R.; Brindley, H. E.; Highwood, E. J.; Marsham, J. H.; Parker, D. J.; Todd, M. C.; Banks, J. R.; Brooke, J. K.; Engelstaedter, S.; Estelles, V.; Formenti, P.; Garcia-Carreras, L.; Kocha, C.; Marenco, F.; Sodemann, H.; Allen, C. J. T.; Bourdon, A.; Bart, M.; Cavazos-Guerra, C.; Chevaillier, S.; Crosier, J.; Darbyshire, E.; Dean, A. R.; Dorsey, J. R.; Kent, J.; O'Sullivan, D.; Schepanski, K.; Szpek, K.; Trembath, J.; Woolley, A.

2015-07-01

The Fennec climate programme aims to improve understanding of the Saharan climate system through a synergy of observations and modelling. We present a description of the Fennec airborne observations during 2011 and 2012 over the remote Sahara (Mauritania and Mali) and the advances in the understanding of mineral dust and boundary layer processes they have provided. Aircraft instrumentation aboard the UK FAAM BAe146 and French SAFIRE (Service des Avions Français Instrumentés pour la Recherche en Environnement) Falcon 20 is described, with specific focus on instrumentation specially developed for and relevant to Saharan meteorology and dust. Flight locations, aims and associated meteorology are described. Examples and applications of aircraft measurements from the Fennec flights are presented, highlighting new scientific results delivered using a synergy of different instruments and aircraft. These include (1) the first airborne measurement of dust particles sizes of up to 300 microns and associated dust fluxes in the Saharan atmospheric boundary layer (SABL), (2) dust uplift from the breakdown of the nocturnal low-level jet before becoming visible in SEVIRI (Spinning Enhanced Visible Infra-Red Imager) satellite imagery, (3) vertical profiles of the unique vertical structure of turbulent fluxes in the SABL, (4) in situ observations of processes in SABL clouds showing dust acting as cloud condensation nuclei (CCN) and ice nuclei (IN) at -15 °C, (5) dual-aircraft observations of the SABL dynamics, thermodynamics and composition in the Saharan heat low region (SHL), (6) airborne observations of a dust storm associated with a cold pool (haboob) issued from deep convection over the Atlas Mountains, (7) the first airborne chemical composition measurements of dust in the SHL region with differing composition, sources (determined using Lagrangian backward trajectory calculations) and absorption properties between 2011 and 2012, (8) coincident ozone and dust surface area measurements suggest coarser particles provide a route for ozone depletion, (9) discrepancies between airborne coarse-mode size distributions and AERONET (AERosol Robotic NETwork) sunphotometer retrievals under light dust loadings. These results provide insights into boundary layer and dust processes in the SHL region - a region of substantial global climatic importance.

Modeling the global emission, transport and deposition of trace elements associated with mineral dust

DOE PAGES

Zhang, Y.; Mahowald, N.; Scanza, R. A.; ...

2015-10-12

Trace element deposition from desert dust has important impacts on ocean primary productivity, the quantification of which could be useful in determining the magnitude and sign of the biogeochemical feedback on radiative forcing. However, the impact of elemental deposition to remote ocean regions is not well understood and is not currently included in global climate models. In this study, emission inventories for eight elements primarily of soil origin, Mg, P, Ca, Mn, Fe, K, Al, and Si are determined based on a global mineral data set and a soil data set. The resulting elemental fractions are used to drive themore » desert dust model in the Community Earth System Model (CESM) in order to simulate the elemental concentrations of atmospheric dust. Spatial variability of mineral dust elemental fractions is evident on a global scale, particularly for Ca. Simulations of global variations in the Ca / Al ratio, which typically range from around 0.1 to 5.0 in soils, are consistent with observations, suggesting that this ratio is a good signature for dust source regions. The simulated variable fractions of chemical elements are sufficiently different; estimates of deposition should include elemental variations, especially for Ca, Al and Fe. The model results have been evaluated with observations of elemental aerosol concentrations from desert regions and dust events in non-dust regions, providing insights into uncertainties in the modeling approach. The ratios between modeled and observed elemental fractions range from 0.7 to 1.6, except for Mg and Mn (3.4 and 3.5, respectively). Using the soil database improves the correspondence of the spatial heterogeneity in the modeling of several elements (Ca, Al and Fe) compared to observations. Total and soluble dust element fluxes to different ocean basins and ice sheet regions have been estimated, based on the model results. The annual inputs of soluble Mg, P, Ca, Mn, Fe and K associated with dust using the mineral data set are 0.30 Tg, 16.89 Gg, 1.32 Tg, 22.84 Gg, 0.068 Tg, and 0.15 Tg to global oceans and ice sheets.« less

Source apportionments of ambient fine particulate matter in Israeli, Jordanian, and Palestinian cities.

PubMed

Heo, Jongbae; Wu, Bo; Abdeen, Ziad; Qasrawi, Radwan; Sarnat, Jeremy A; Sharf, Geula; Shpund, Kobby; Schauer, James J

2017-06-01

This manuscript evaluates spatial and temporal variations of source contributions to ambient fine particulate matter (PM 2.5 ) in Israeli, Jordanian, and Palestinian cities. Twenty-four hour integrated PM 2.5 samples were collected every six days over a 1-year period (January to December 2007) in four cities in Israel (West Jerusalem, Eilat, Tel Aviv, and Haifa), four cities in Jordan (Amman, Aqaba, Rahma, and Zarka), and three cities in Palestine (Nablus, East Jerusalem, and Hebron). The PM 2.5 samples were analyzed for major chemical components, including organic carbon and elemental carbon, ions, and metals, and the results were used in a positive matrix factorization (PMF) model to estimate source contributions to PM 2.5 mass. Nine sources, including secondary sulfate, secondary nitrate, mobile, industrial lead sources, dust, construction dust, biomass burning, fuel oil combustion and sea salt, were identified across the sampling sites. Secondary sulfate was the dominant source, contributing 35% of the total PM 2.5 mass, and it showed relatively homogeneous temporal trends of daily source contribution in the study area. Mobile sources were found to be the second greatest contributor to PM 2.5 mass in the large metropolitan cities, such as Tel Aviv, Hebron, and West and East Jerusalem. Other sources (i.e. industrial lead sources, construction dust, and fuel oil combustion) were closely related to local emissions within individual cities. This study demonstrates how international cooperation can facilitate air pollution studies that address regional air pollution issues and the incremental differences across cities in a common airshed. It also provides a model to study air pollution in regions with limited air quality monitoring capacity that have persistent and emerging air quality problems, such as Africa, South Asia and Central America. Copyright © 2017 Elsevier Ltd. All rights reserved.

Sources of PM10 Air Pollution in Rural Area in the Vicinity of a Highway In Žilina Selfgoverning Region, Slovakia

NASA Astrophysics Data System (ADS)

Jandačka, Dušan

2015-05-01

Particulate matter results as an aftermath of numerous distinctive processes in the atmosphere and they become a part of everyday life. Their harmful effect and impact on the ambient environment is determined predominantly by the presence of various chemical substances and elements. The chemical composition of these particles (organic and elemental carbon, mineral dust, sea aerosols, secondary particles, especially sulphates and nitrates, heavy metals and further elements) is mainly impacted on by their origin, whereas the primary source of the particulate matter is determined and specified by the profile of chemical elements and substances. Particulate Matter (PM) may originate in various natural resources or anthropogenic sources. Among the natural sources sea salt is to be counted on, dust of the earth crust, pollen and volcanic ashes. Anthropogenic sources do include, predominantly, burning fossil fuels in the fossil-fuel power plants, local heating of households, burning liquefied fossil fuels in the combustion engines of vehicles, noncombustion related emissions as a result of vehicular traffic, resuspension of the road-traffic-related dust.

Global trends in visibility: Implications for dust sources

USGS Publications Warehouse

Mahowald, N.M.; Ballantine, J.A.; Feddema, J.; Ramankutty, N.

2007-01-01

There is a large uncertainty in the relative roles of human land use, climate change and carbon dioxide fertilization in changing desert dust source strength over the past 100 years, and the overall sign of human impacts on dust is not known. We used visibility data from meteorological stations in dusty regions to assess the anthropogenic impact on long term trends in desert dust emissions. We did this by looking at time series of visibility derived variables and their correlations with precipitation, drought, winds, land use and grazing. Visibility data are available at thousands of stations globally from 1900 to the present, but we focused on 357 stations with more than 30 years of data in regions where mineral aerosols play a dominant role in visibility observations. We evaluated the 1974 to 2003 time period because most of these stations have reliable records only during this time. We first evaluated the visibility data against AERONET aerosol optical depth data, and found that only in dusty regions are the two moderately correlated. Correlation coefficients between visibility-derived variables and AERONET optical depths indicate a moderate correlation (0.47), consistent with capturing about 20% of the variability in optical depths. Two visibility-derived variables appear to compare the best with AERONET observations: the fraction of observations with visibility less than 5 km (VIS5) and the surface extinction (EXT). Regional trends show that in many dusty places, VIS5 and EXT are statistically significantly correlated with the Palmer drought severity index (based on precipitation and temperature) or surface wind speeds, consistent with dust temporal variability being largely driven by meteorology. This is especially true for North African and Chinese dust sources, but less true in the Middle East, Australia or South America, where there are not consistent patterns in the correlations. Climate indices such as El Nino or the North Atlantic Oscillation are not correlated with visibility-derived variables in this analysis. There are few stations where visibility measures are correlated with cultivation or grazing estimates on a temporal basis, although this may be a function of the very coarse temporal resolution of the land use datasets. On the other hand, spatial analysis of the visibility data suggests that natural topographic lows are not correlated with VIS5 or EXT, but land use is correlated at a moderate level. This analysis is consistent with land use being important in some regions, but meteorology driving interannual variability during 1974-2003.

Determining the infrared radiative effects of Saharan dust: a radiative transfer modelling study based on vertically resolved measurements at Lampedusa

NASA Astrophysics Data System (ADS)

Meloni, Daniela; di Sarra, Alcide; Brogniez, Gérard; Denjean, Cyrielle; De Silvestri, Lorenzo; Di Iorio, Tatiana; Formenti, Paola; Gómez-Amo, José L.; Gröbner, Julian; Kouremeti, Natalia; Liuzzi, Giuliano; Mallet, Marc; Pace, Giandomenico; Sferlazzo, Damiano M.

2018-03-01

Detailed measurements of radiation, atmospheric and aerosol properties were carried out in summer 2013 during the Aerosol Direct Radiative Impact on the regional climate in the MEDiterranean region (ADRIMED) campaign in the framework of the Chemistry-Aerosol Mediterranean Experiment (ChArMEx) experiment. This study focusses on the characterization of infrared (IR) optical properties and direct radiative effects of mineral dust, based on three vertical profiles of atmospheric and aerosol properties and IR broadband and narrowband radiation from airborne measurements, made in conjunction with radiosonde and ground-based observations at Lampedusa, in the central Mediterranean. Satellite IR spectra from the Infrared Atmospheric Sounder Interferometer (IASI) are also included in the analysis. The atmospheric and aerosol properties are used as input to a radiative transfer model, and various IR radiation parameters (upward and downward irradiance, nadir and zenith brightness temperature at different altitudes) are calculated and compared with observations. The model calculations are made for different sets of dust particle size distribution (PSD) and refractive index (RI), derived from observations and from the literature. The main results of the analysis are that the IR dust radiative forcing is non-negligible and strongly depends on PSD and RI. When calculations are made using the in situ measured size distribution, it is possible to identify the refractive index that produces the best match with observed IR irradiances and brightness temperatures (BTs). The most appropriate refractive indices correspond to those determined from independent measurements of mineral dust aerosols from the source regions (Tunisia, Algeria, Morocco) of dust transported over Lampedusa, suggesting that differences in the source properties should be taken into account. With the in situ size distribution and the most appropriate refractive index the estimated dust IR radiative forcing efficiency is +23.7 W m-2 at the surface, -7.9 W m-2 within the atmosphere, and +15.8 W m-2 at the top of the atmosphere. The use of column-integrated dust PSD from AERONET may also produce a good agreement with measured irradiances and BTs, but with significantly different values of the RI. This implies large differences, up to a factor of 2.5 at surface, in the estimated dust radiative forcing, and in the IR heating rate. This study shows that spectrally resolved measurements of BTs are important to better constrain the dust IR optical properties, and to obtain a reliable estimate of its radiative effects. Efforts should be directed at obtaining an improved description of the dust size distribution and its vertical distribution, as well as at including regionally resolved optical properties.

Source apportionment and health risk assessment of potentially toxic elements in road dust from urban industrial areas of Ahvaz megacity, Iran.

PubMed

Najmeddin, Ali; Keshavarzi, Behnam; Moore, Farid; Lahijanzadeh, Ahmadreza

2017-10-28

This study investigates the occurrence and spatial distribution of potentially toxic elements (PTEs) (Hg, Cd, Cu, Mo, Pb, Zn, Ni, Co, Cr, Al, Fe, Mn, V and Sb) in 67 road dust samples collected from urban industrial areas in Ahvaz megacity, southwest of Iran. Geochemical methods, multivariate statistics, geostatistics and health risk assessment model were adopted to study the spatial pollution pattern and to identify the priority pollutants, regions of concern and sources of the studied PTEs. Also, receptor positive matrix factorization model was employed to assess pollution sources. Compared to the local background, the median enrichment factor values revealed the following order: Sb > Pb > Hg > Zn > Cu > V > Fe > Mo > Cd > Mn > Cr ≈ Co ≈ Al ≈ Ni. Statistical results show that a significant difference exists between concentrations of Mo, Cu, Pb, Zn, Fe, Sb, V and Hg in different regions (univariate analysis, Kruskal-Wallis test p < 0.05), indicating the existence of highly contaminated spots. Integrated source identification coupled with positive matrix factorization model revealed that traffic-related emissions (43.5%) and steel industries (26.4%) were first two sources of PTEs in road dust, followed by natural sources (22.6%) and pipe and oil processing companies (7.5%). The arithmetic mean of pollution load index (PLI) values for high traffic sector (1.92) is greater than industrial (1.80) and residential areas (1.25). Also, the results show that ecological risk values for Hg and Pb in 41.8 and 9% of total dust samples are higher than 80, indicating their considerable or higher potential ecological risk. The health risk assessment model showed that ingestion of dust particles contributed more than 83% of the overall non-carcinogenic risk. For both residential and industrial scenarios, Hg and Pb had the highest risk values, whereas Mo has the lowest value.

Impacts of interactive dust and its direct radiative forcing on interannual variations of temperature and precipitation in winter over East Asia: Impacts of Dust on IAVs of Temperature

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lou, Sijia; Russell, Lynn M.; Yang, Yang

We used 150-year pre-industrial simulations of the Community Earth System Model (CESM) to quantify the impacts of interactively-modeled dust emissions on the interannual variations of temperature and precipitation over East Asia during the East Asian Winter Monsoon (EAWM) season. The simulated December-January-February dust column burden and dust optical depth are lower over northern China in the strongest EAWM years than those of the weakest years, with regional mean values lower by 38.3% and 37.2%, respectively. The decrease in dust over the dust source regions (the Taklamakan and Gobi Deserts) and the downwind region (such as the North China Plain) leadsmore » to an increase in direct radiative forcing (RF) both at the surface and top of atmosphere by up to 1.5 and 0.75 W m-2, respectively. The effects of EAWM-related variations in surface winds, precipitation and their effects on dust emissions and wet removal contribute about 67% to the total dust-induced variations of direct RF at the surface and partly offset the cooling that occurs with the EAWM strengthening by heating the surface. The variations of surface air temperature induced by the changes in wind and dust emissions increase by 0.4-0.6 K over eastern coastal China, northeastern China, and Japan, which weakens the impact of EAWM on surface air temperature by 3–18% in these regions. The warming results from the combined effects of changes in direct RF and easterly wind anomalies that bring warm air from the ocean to these regions. Moreover, the feedback of the changes in wind on dust emissions weakens the variations of the sea level pressure gradient on the Siberian High while enhancing the Maritime Continent Low. Therefore, cold air is prevented from being transported from Siberia, Kazakhstan, western and central China to the western Pacific Ocean and decreases surface air temperature by 0.6 K and 2 K over central China and the Tibetan Plateau, respectively. Over eastern coastal China, the variations of large-scale precipitation induced by the feedback of EAWM-related changes in wind on dust emissions increase by 10-30% in winter because of the increase in surface air temperature and the anomalous circulation.« less

Data Release of UV to Submillimeter Broadband Fluxes for Simulated Galaxies from the EAGLE Project

NASA Astrophysics Data System (ADS)

Camps, Peter; Trčka, Ana; Trayford, James; Baes, Maarten; Theuns, Tom; Crain, Robert A.; McAlpine, Stuart; Schaller, Matthieu; Schaye, Joop

2018-02-01

We present dust-attenuated and dust emission fluxes for sufficiently resolved galaxies in the EAGLE suite of cosmological hydrodynamical simulations, calculated with the SKIRT radiative transfer code. The post-processing procedure includes specific components for star formation regions, stellar sources, and diffuse dust and takes into account stochastic heating of dust grains to obtain realistic broadband fluxes in the wavelength range from ultraviolet to submillimeter. The mock survey includes nearly half a million simulated galaxies with stellar masses above {10}8.5 {M}ȯ across six EAGLE models. About two-thirds of these galaxies, residing in 23 redshift bins up to z = 6, have a sufficiently resolved metallic gas distribution to derive meaningful dust attenuation and emission, with the important caveat that the same dust properties were used at all redshifts. These newly released data complement the already publicly available information about the EAGLE galaxies, which includes intrinsic properties derived by aggregating the properties of the smoothed particles representing matter in the simulation. We further provide an open-source framework of Python procedures for post-processing simulated galaxies with the radiative transfer code SKIRT. The framework allows any third party to calculate synthetic images, spectral energy distributions, and broadband fluxes for EAGLE galaxies, taking into account the effects of dust attenuation and emission.

Radiative Energetics of Mineral Dust Aerosols from Ground-Based Measurements

NASA Technical Reports Server (NTRS)

Tsay, Si-Chee; Hansell, Richard A.

2011-01-01

Airborne dust aerosols worldwide contribute a significant part to air quality problems and, to some extent, regional climatic issues (e.g., radiative forcing, hydrological cycle, and primary biological productivity in oceans). Evaluating the direct solar radiative effect of dust aerosols is relatively straightforward due in part to the relatively large SIN ratio in broadband irradiance measurements. The longwave (LW) impact, on the other hand, is rather difficult to ascertain since the measured dust signal level (approx.10 W/sq m) is on the same order as the instrumental uncertainties. Although the magnitude of the LW impact is much smaller than that of the shortwave (SW), it can still have a noticeable influence on the energy distribution of Earth-atmosphere system, particularly due to the strong light-absorptive properties commonly found in many terrestrial minerals. The current effort is part of an ongoing research study to perform a global assessment of dust direct aerosol radiative effects (DARE) during major field deployments of key dust source regions worldwide. In this work we present results stemming from two previous field deployments: the 2006 NASA African Monsoon Multidisciplinary Activities and the 2008 Asian Monsoon Years, both utilizing NASA Goddard's mobile ground-based facility. The former study focused on transported Saharan dust at Sal (16.73degN, 22.93degW), Cape Verde along the west coast of Africa while the latter focused on Asian dust at Zhangye (39.082degN, 100.276degE), China near the source between the Taklimakan and Gobi deserts. Due to the compelling variability in spatial and temporal scale of dust properties during field experiments, a deterministic I-D radiative transfer model constrained by local measurements (i.e., spectral photometry/interferometry and lidar for physical/microphysical, mineralogy, and single-scattering properties) is employed to evaluate dust's local instantaneous SW/LW DARE both at the surface and at the top of the atmosphere along with heating rate profiles for cloud-free atmospheres. In both dust cases the efficiency in the L W DARE is investigated and its significance is compared relative to that of diurnally SW.

Numerical simulation of "An American Haboob"

NASA Astrophysics Data System (ADS)

Vukovic, A.; Vujadinovic, M.; Pejanovic, G.; Andric, J.; Kumjian, M. R.; Djurdjevic, V.; Dacic, M.; Prasad, A. K.; El-Askary, H. M.; Paris, B. C.; Petkovic, S.; Nickovic, S.; Sprigg, W. A.

2013-10-01

A dust storm of fearful proportions hit Phoenix in the early evening hours of 5 July 2011. This storm, an American haboob, was predicted hours in advance because numerical, land-atmosphere modeling, computing power and remote sensing of dust events have improved greatly over the past decade. High resolution numerical models are required for accurate simulation of the small-scales of the haboob process, with high velocity surface winds produced by strong convection and severe downbursts. Dust productive areas in this region consist mainly of agricultural fields, with soil surfaces disturbed by plowing and tracks of land in the high Sonoran desert laid barren by ongoing draught. Model simulation of the 5 July 2011 dust storm uses the coupled atmospheric-dust model NMME-DREAM with 3.5 km horizontal resolution. A mask of the potentially dust productive regions is obtained from the land cover and the Normalized Difference Vegetation Index (NDVI) data from the Moderate Resolution Imaging Spectroradiometer (MODIS). Model results are compared with radar and other satellite-based images and surface meteorological and PM10 observations. The atmospheric model successfully hindcasted the position of the front in space and time, with about 1 h late arrival in Phoenix. The dust model predicted the rapid uptake of dust and high values of dust concentration in the ensuing storm. South of Phoenix, over the closest source regions (~ 25 km), the model PM10 surface dust concentration reached ~ 2500 μg m-3, but underestimated the values measured by the PM10stations within the city. Model results are also validated by the MODIS aerosol optical depth (AOD), employing deep blue (DB) algorithms for aerosol loadings. Model validation included Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO), equipped with the lidar instrument, to disclose the vertical structure of dust aerosols as well as aerosol subtypes. Promising results encourage further research and application of high-resolution modeling and satellite-based remote sensing to warn of approaching severe dust events and reduce risks for safety and health.

Asian Dust Storm Outbreaks: A Satellite-Surface Perspective

NASA Technical Reports Server (NTRS)

Tsay, Si-Chee

2006-01-01

Airborne dusts from northern China contribute a significant part of the air quality problem and, to some extent, regional climatic impact in Asia during springtime. Asian dust typically originates in desert areas far from polluted urban regions. During the transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian dust is of special importance in regional-to-global climate issues (e.g., radiative forcing, hydrological cycle, and primary biological productivity in the mid-Pacific Ocean, etc.), as well as societal concerns (e.g., adverse health effects to humans). The Asian dust and air pollution aerosols can be detected by its colored appearance on current Earth observing satellites (e.g., MODIS, SeaWiFS, TOMS, etc.) and its evolution monitored by satellites and surface network (e.g. AERONET, SKY NET, MPLNET, etc.). Recently, many field campaigns (e.g., ACE-Asia-2001, TRACEP-2001, ADE-2002 & -2003, APEX-2001 & -2003, etc.) were designed and executed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentrations over eastern Asia and along the rim of the western Pacific. I will present an overview of the outbreak of Asian dust storms from space and surface observations and to address the climatic effects and societal impacts.

IRAS 21391 + 5802 - A study in intermediate mass star formation

NASA Technical Reports Server (NTRS)

Wilking, Bruce; Mundy, Lee; Mcmullin, Joseph; Hezel, Thomas; Keene, Jocelyn

1993-01-01

We present infrared and millimeter wavelength observations of the cold IRAS source 21391 + 5802 and its associated molecular core. Infrared observations at lambda = 3.5 microns reveal a heavily obscured, central point source which is coincident with a compact lambda = 2.7 mm continuum and C18O emission region. The source radiates about 310 solar luminosities, primarily at FIR wavelengths, suggesting that it is a young stellar object of intermediate mass. The steeply rising spectral energy distribution and the large fraction of the system mass residing in circumstellar material imply that IRAS 21391 + 5802 is in an early stage of evolution. The inferred dust temperature indicates a temperature gradient in the core. A comprehensive model for the surrounding core of dust and gas is devised to match the observed dust continuum emission and multitransition CS emission from this and previous studies. We find a r exp -1.5 +/- 0.2 density gradient consistent with that of a gravitationally evolved core and a total core mass of 380 solar masses. The observed dust emission is most consistent with a lambda exp -1.5 - lambda exp -2 dust emissivity law; for a lambda exp -2 law, the data are best fit by a mass opacity coefficient of 3.6 x 10 exp -3 sq cm/g at lambda = 1.25 mm.

Large Salt Dust Storms Follow a 30-Year Rainfall Cycle in the Mar Chiquita Lake (Córdoba, Argentina)

PubMed Central

Stein, Ariel F.

2016-01-01

Starting in 2006, a new source of intense salt dust storms developed in Mar Chiquita (Córdoba, Argentina), the largest saline lake in South America. Storms originate from vast mudflats left by a 30-year expansion-retreat cycle of the lake due to changes in the regional rainfall regime. The annual frequency of salt dust storms correlated with the size of the salt mudflats. Events were restricted to the coldest months, and reached up to 800 km from the source. Occurrence of dust storms was associated with specific surface colors and textures easily identifiable in satellite images. High-emission surfaces were characterized by the presence of sodium sulfate hydrous/anhydrous crystals (mirabilite and thenardite), and a superficial and variable water table, which may result in the periodic development of a characteristic “fluffy” surface derived from salt precipitation-dissolution processes. HYSPLIT model simulation estimates a deposition maximum near the sources (of about 2.5 kg/ha/yr), and a decreasing trend from the emission area outwards, except for the relative secondary maximum modeled over the mountain ranges in southern Bolivia and northern Argentina due to an orographic effect. The 2009 total deposition of salt dust generated in Mar Chiquita was estimated at 6.5 million tons. PMID:27258088

Large Salt Dust Storms Follow a 30-Year Rainfall Cycle in the Mar Chiquita Lake (Córdoba, Argentina).

PubMed

Bucher, Enrique H; Stein, Ariel F

2016-01-01

Starting in 2006, a new source of intense salt dust storms developed in Mar Chiquita (Córdoba, Argentina), the largest saline lake in South America. Storms originate from vast mudflats left by a 30-year expansion-retreat cycle of the lake due to changes in the regional rainfall regime. The annual frequency of salt dust storms correlated with the size of the salt mudflats. Events were restricted to the coldest months, and reached up to 800 km from the source. Occurrence of dust storms was associated with specific surface colors and textures easily identifiable in satellite images. High-emission surfaces were characterized by the presence of sodium sulfate hydrous/anhydrous crystals (mirabilite and thenardite), and a superficial and variable water table, which may result in the periodic development of a characteristic "fluffy" surface derived from salt precipitation-dissolution processes. HYSPLIT model simulation estimates a deposition maximum near the sources (of about 2.5 kg/ha/yr), and a decreasing trend from the emission area outwards, except for the relative secondary maximum modeled over the mountain ranges in southern Bolivia and northern Argentina due to an orographic effect. The 2009 total deposition of salt dust generated in Mar Chiquita was estimated at 6.5 million tons.

Theory of Dust Voids in Plasmas

NASA Technical Reports Server (NTRS)

Goree, J.; Morfill, G. E.; Tsytovich, V. N.; Vladimirov, S. V.

1999-01-01

Dusty plasmas in a gas discharge often feature a stable void, i.e., a dust-free region inside the dust cloud. This occurs under conditions relevant to both plasma processing discharges and plasma crystal experiments. The void results from a balance of the electrostatic and ion drag forces on a dust particle. The ion drag force is driven by a flow of ions outward from an ionization source and toward the surrounding dust cloud, which has a negative space charge. In equilibrium the force balance for dust particles requires that the boundary with the dust cloud be sharp, provided that the particles are cold and monodispersive. Numerical solutions of the one-dimensional nonlinear fluid equations are carried out including dust charging and dust-neutral collisions, but not ion-neutral collisions. The regions of parameter space that allow stable void equilibria are identified. There is a minimum ionization rate that can sustain a void. Spatial profiles of plasma parameters in the void are reported. In the absence of ion-neutral collisions, the ion flow enters the dust cloud's edge at Mach number M = 1. Phase diagrams for expanding or contracting voids reveal a stationary point corresponding to a single stable equilibrium void size, provided the ionization rate is constant. Large voids contract and small voids expand until they attain this stationary void size. On the other hand, if the ionization rate is not constant, the void size can oscillate. Results are compared to recent laboratory and microgravity experiments.

Determining the Influence of Dust on Post-Glacial Lacustrine Sedimentation in Bald Lake, Uinta Mountains, Utah

NASA Astrophysics Data System (ADS)

O'Keefe, S. S.; McElroy, R.; Munroe, J. S.

2016-12-01

Dust is increasingly recognized as an important component of biogeochemical cycling and ecosystem function in mountain environments. Previous work has shown that delivery of dust to the Uinta Mountains of northeastern Utah has influenced pedogenesis, soil nutrient status, and surface water chemistry. An array of passive and active samplers in the alpine zone of the Uintas provides detailed information about contemporary dust fluxes, along with physical and geochemical properties of modern dust. Reconstruction of changes in the dust system over time, however, requires continuous sedimentary archives sensitive to dust inputs. A radiocarbon-dated 3.5-m core (spanning 12.7 kyr) collected from subalpine Bald Lake may provide such a record. Passive dust collectors in the vicinity of the lake constrain the geochemical properties of modern dust, whereas samples of regolith constrain properties of the local surficial material within the watershed. Together, these represent two end member sources of clastic sediment to Bald Lake basin: allochthonous dust and autochthonous regolith. Ba and Eu are found in higher abundances in the dust than in the watershed regolith. Zr and Th are found to be lower in the dust than in the watershed. Geochemical analysis of the sediment core allows the relative contribution of exotic and local material to the lake to be considered as a time series covering the post-glacial interval when indicator elements are plotted. Findings suggest Bald Lake's dust record tracks regional aridity and corresponds to low-stands of large lakes in the southwestern United States. Spatial variability of elemental abundances in the watershed suggests there are more than two input sources contributing to the lake over time.

ABSENCE OF SIGNIFICANT COOL DISKS IN YOUNG STELLAR OBJECTS EXHIBITING REPETITIVE OPTICAL OUTBURSTS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Hauyu Baobab; Hirano, Naomi; Takami, Michihiro

2016-01-10

We report Submillimeter Array 1.3 mm high angular resolution observations toward the four EXor-type outbursting young stellar objects VY Tau, V1118 Ori, V1143 Ori, and NY Ori. The data mostly show low dust masses M{sub dust} in the associated circumstellar disks. Among the sources, NY Ori possesses a relatively massive disk with M{sub dust} ∼ 9 × 10{sup −4}M{sub ⊙}. V1118 Ori has a marginal detection equivalent to M{sub dust} ∼ 6 × 10{sup −5}M{sub ⊙}. V1143 Ori has a non-detection also equivalent to M{sub dust} < 6 × 10{sup −5}M{sub ⊙}. For the nearest source, VY Tau, we get a surprising non-detection that provides a stringent upper limit M{sub dust} < 6 × 10{sup −6}M{sub ⊙}.more » We interpret our findings as suggesting that the gas and dust reservoirs that feed the short-duration, repetitive optical outbursts seen in some EXors may be limited to the small-scale, innermost region of their circumstellar disks. This hot dust may have escaped our detection limits. Follow-up, more sensitive millimeter observations are needed to improve our understanding of the triggering mechanisms of EXor-type outbursts.« less

Parameterization of dust emissions in the global atmospheric chemistry-climate model EMAC: impact of nudging and soil properties

NASA Astrophysics Data System (ADS)

Astitha, M.; Lelieveld, J.; Abdel Kader, M.; Pozzer, A.; de Meij, A.

2012-11-01

Airborne desert dust influences radiative transfer, atmospheric chemistry and dynamics, as well as nutrient transport and deposition. It directly and indirectly affects climate on regional and global scales. Two versions of a parameterization scheme to compute desert dust emissions are incorporated into the atmospheric chemistry general circulation model EMAC (ECHAM5/MESSy2.41 Atmospheric Chemistry). One uses a globally uniform soil particle size distribution, whereas the other explicitly accounts for different soil textures worldwide. We have tested these two versions and investigated the sensitivity to input parameters, using remote sensing data from the Aerosol Robotic Network (AERONET) and dust concentrations and deposition measurements from the AeroCom dust benchmark database (and others). The two versions are shown to produce similar atmospheric dust loads in the N-African region, while they deviate in the Asian, Middle Eastern and S-American regions. The dust outflow from Africa over the Atlantic Ocean is accurately simulated by both schemes, in magnitude, location and seasonality. Approximately 70% of the modelled annual deposition data and 70-75% of the modelled monthly aerosol optical depth (AOD) in the Atlantic Ocean stations lay in the range 0.5 to 2 times the observations for all simulations. The two versions have similar performance, even though the total annual source differs by ~50%, which underscores the importance of transport and deposition processes (being the same for both versions). Even though the explicit soil particle size distribution is considered more realistic, the simpler scheme appears to perform better in several locations. This paper discusses the differences between the two versions of the dust emission scheme, focusing on their limitations and strengths in describing the global dust cycle and suggests possible future improvements.

Characterizing the annual cycle of African dust transport to the Caribbean Basin and South America and its impact on the environment and air quality

NASA Astrophysics Data System (ADS)

Prospero, Joseph M.; Collard, François-Xavier; Molinié, Jack; Jeannot, Alexis

2014-07-01

Decades of aerosol measurements on Barbados have yielded a detailed picture of African mineral dust transport to the Caribbean Basin that shows a strong seasonal cycle with a maximum in boreal summer and a minimum in winter. Satellite aerosol products suggest that in spring, there is a comparable transport to northeastern South America. Here we characterize the complete annual cycle of dust transport to the western Atlantic by linking the Barbados record to multiyear records of airborne particulate matter less than 10 µm diameter (PM10) measured in air quality programs at Cayenne (French Guiana) and Guadeloupe. Comparisons of PM10 at these sites with concurrent dust measurements at Barbados demonstrate that high PM10 levels are almost entirely due to dust. Cayenne PM10 peaks in spring in a cycle which is consistent with satellite aerosol optical depth and suggests that the Sahel is the dominant source. The persistent transport of dust during much of the year could impact a wide range of environmental processes over a broad region that extends from the southern United States to the Amazon Basin. Finally, the average 24 h PM10 concentrations at Cayenne and Guadeloupe frequently exceed the World Health Organization air quality guideline. Thus soil dust PM10 could be a significant, but generally unrecognized, health factor at western Atlantic sites and also in other relatively remote regions affected by long-range dust from Africa. Because dust emissions and transport are highly sensitive to climate variability, climate change in coming decades could greatly affect a wide range of biogeochemical processes and human health in this region.

Integration of Dust Prediction Systems and Vegetation Phenology to Track Pollen for Asthma Alerts in Public Health

NASA Technical Reports Server (NTRS)

Luvall, Jeffrey C.; Sprigg, W. A.; Huete, A.; Nickovic, S.; Pejanovic, G.; Levetin, E.; Van de water, P.; Myers, O.; Budge, A. M.; Krapfl, H.;

Simulation of windblown dust transport from a mine tailings impoundment using a computational fluid dynamics model

NASA Astrophysics Data System (ADS)

Stovern, Michael; Felix, Omar; Csavina, Janae; Rine, Kyle P.; Russell, MacKenzie R.; Jones, Robert M.; King, Matt; Betterton, Eric A.; Sáez, A. Eduardo

2014-09-01

Mining operations are potential sources of airborne particulate metal and metalloid contaminants through both direct smelter emissions and wind erosion of mine tailings. The warmer, drier conditions predicted for the Southwestern US by climate models may make contaminated atmospheric dust and aerosols increasingly important, due to potential deleterious effects on human health and ecology. Dust emissions and dispersion of dust and aerosol from the Iron King Mine tailings in Dewey-Humboldt, Arizona, a Superfund site, are currently being investigated through in situ field measurements and computational fluid dynamics modeling. These tailings are heavily contaminated with lead and arsenic. Using a computational fluid dynamics model, we model dust transport from the mine tailings to the surrounding region. The model includes gaseous plume dispersion to simulate the transport of the fine aerosols, while individual particle transport is used to track the trajectories of larger particles and to monitor their deposition locations. In order to improve the accuracy of the dust transport simulations, both regional topographical features and local weather patterns have been incorporated into the model simulations. Results show that local topography and wind velocity profiles are the major factors that control deposition.

Simulation of windblown dust transport from a mine tailings impoundment using a computational fluid dynamics model.

PubMed

Stovern, Michael; Felix, Omar; Csavina, Janae; Rine, Kyle P; Russell, MacKenzie R; Jones, Robert M; King, Matt; Betterton, Eric A; Sáez, A Eduardo

2014-09-01

Mining operations are potential sources of airborne particulate metal and metalloid contaminants through both direct smelter emissions and wind erosion of mine tailings. The warmer, drier conditions predicted for the Southwestern US by climate models may make contaminated atmospheric dust and aerosols increasingly important, due to potential deleterious effects on human health and ecology. Dust emissions and dispersion of dust and aerosol from the Iron King Mine tailings in Dewey-Humboldt, Arizona, a Superfund site, are currently being investigated through in situ field measurements and computational fluid dynamics modeling. These tailings are heavily contaminated with lead and arsenic. Using a computational fluid dynamics model, we model dust transport from the mine tailings to the surrounding region. The model includes gaseous plume dispersion to simulate the transport of the fine aerosols, while individual particle transport is used to track the trajectories of larger particles and to monitor their deposition locations. In order to improve the accuracy of the dust transport simulations, both regional topographical features and local weather patterns have been incorporated into the model simulations. Results show that local topography and wind velocity profiles are the major factors that control deposition.

A Broad 22 Micron Emission Feature in the Carina Nebula H ii Region.

PubMed

Chan; Onaka

2000-04-10

We report the detection of a broad 22 µm emission feature in the Carina Nebula H ii region by the Infrared Space Observatory (ISO) short-wavelength spectrometer. The feature shape is similar to that of the 22 µm emission feature of newly synthesized dust observed in the Cassiopeia A supernova remnant. This finding suggests that both of the features are arising from the same carrier and that supernovae are probably the dominant production sources of this new interstellar grain. A similar broad emission dust feature is also found in the spectra of two starburst galaxies from the ISO archival data. This new dust grain could be an abundant component of interstellar grains and can be used to trace the supernova rate or star formation rate in external galaxies. The existence of the broad 22 µm emission feature complicates the dust model for starburst galaxies and must be taken into account correctly in the derivation of dust color temperature. Mg protosilicate has been suggested as the carrier of the 22 µm emission dust feature observed in Cassiopeia A. The present results provide useful information in studies on the chemical composition and emission mechanism of the carrier.

Simulation of windblown dust transport from a mine tailings impoundment using a computational fluid dynamics model

PubMed Central

Stovern, Michael; Felix, Omar; Csavina, Janae; Rine, Kyle P.; Russell, MacKenzie R.; Jones, Robert M.; King, Matt; Betterton, Eric A.; Sáez, A. Eduardo

2014-01-01

Mining operations are potential sources of airborne particulate metal and metalloid contaminants through both direct smelter emissions and wind erosion of mine tailings. The warmer, drier conditions predicted for the Southwestern US by climate models may make contaminated atmospheric dust and aerosols increasingly important, due to potential deleterious effects on human health and ecology. Dust emissions and dispersion of dust and aerosol from the Iron King Mine tailings in Dewey-Humboldt, Arizona, a Superfund site, are currently being investigated through in situ field measurements and computational fluid dynamics modeling. These tailings are heavily contaminated with lead and arsenic. Using a computational fluid dynamics model, we model dust transport from the mine tailings to the surrounding region. The model includes gaseous plume dispersion to simulate the transport of the fine aerosols, while individual particle transport is used to track the trajectories of larger particles and to monitor their deposition locations. In order to improve the accuracy of the dust transport simulations, both regional topographical features and local weather patterns have been incorporated into the model simulations. Results show that local topography and wind velocity profiles are the major factors that control deposition. PMID:25621085

Substantial dust loss of bioavailable phosphorus from agricultural soils

NASA Astrophysics Data System (ADS)

Katra, Itzhak; Gross, Avner; Swet, Nitzan; Tanner, Smadar; Krasnov, Helena; Angert, Alon

2016-04-01

Phosphorus (P) is an essential element in terrestrial ecosystems. Knowledge on the role of dust in the biogeochemical cycling of phosphorus is very limited with no quantitative information on aeolian (by wind) P fluxes from soils. The aim of this study is to focus on P cycling via dust emissions under common land-use practices in an arid environment by integration of sample analyses and aeolian experiments. The experiments indicate significant P fluxes by PM10 dust due to agricultural land use. Even in a single wind-dust event at moderate velocity (7.0 m s-1), P flux in conventional agricultural fields can reach 1.83 kg km-2, that accumulates to a considerable amount per year at a regional scale. The results highlight a negative yearly balance in P content (up to hundreds kg km-2) in all agricultural soils, and thus more P nutrition is required to maintain efficient yield production. In grazing areas where no P nutrition is applied, the soil degradation process can lead to desertification. Emission of P from soil dust sources has significant implications for soil nutrient resources and management strategies in agricultural regions as well as for loading to the atmosphere and global biogeochemical cycles.

Coarse-grained Mineral Dust Deposition in Alpine Lake Sediments: Implications for Regional Drought Patterns and Land-use Changes in the Southwest USA

NASA Astrophysics Data System (ADS)

Pedraza, A.; Kingsley, C.; Marchitto, T. M., Jr.; Lora, J. M.; Pollen, A.; Vollmer, T.; Leithold, E. L.; Mitchell, J.; Tripati, A. K.; Bhattacharya, A.

2017-12-01

Mineral dust accumulation is often causally associated with aridity. However, the relation might not be as straightforward. Consideration of grain sizes and geochemical fingerprinting of the coarse grain fraction will clearly have an impact on how we interpret the sedimentary record of mineral dust in depositional environments e.g. coarse grain fractions of mineral dust would most certainly be transported over relatively short distances and as such in depositional environments, the depositional rate of coarse grains must be determined in order to reliably understand erosional patterns associated with meteorological events (such as frequency of intense wind events such as tornadoes), climatological phenomenon (such as regional droughts) as well as more recently land-use changes. In this study we separate the two size fractions of mineral dust accumulation- fine fraction (typically <4 microns) and coarse fraction (typically >25 microns using grain size analysis from well-studied cores collected from several lake sites distributed across the western southwestern and the Great Plain regions; furthermore we use trace element analysis in each size fraction to identify contributing source regions. We find evidence that the coarser-grain size fraction in the studied lake cores could be of regional origin (and not just local in orgin);. the coarser fraction also appears to be related to intense meteorological events (i.e., the occurrence of cyclones). Analysis is underway to understand the impact of land-use changes on coarse grain fraction

Size-segregated compositional analysis of aerosol particles collected in the European Arctic during the ACCACIA campaign

NASA Astrophysics Data System (ADS)

Young, G.; Jones, H. M.; Darbyshire, E.; Baustian, K. J.; McQuaid, J. B.; Bower, K. N.; Connolly, P. J.; Gallagher, M. W.; Choularton, T. W.

2016-03-01

Single-particle compositional analysis of filter samples collected on board the Facility for Airborne Atmospheric Measurements (FAAM) BAe-146 aircraft is presented for six flights during the springtime Aerosol-Cloud Coupling and Climate Interactions in the Arctic (ACCACIA) campaign (March-April 2013). Scanning electron microscopy was utilised to derive size-segregated particle compositions and size distributions, and these were compared to corresponding data from wing-mounted optical particle counters. Reasonable agreement between the calculated number size distributions was found. Significant variability in composition was observed, with differing external and internal mixing identified, between air mass trajectory cases based on HYbrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) analyses. Dominant particle classes were silicate-based dusts and sea salts, with particles notably rich in K and Ca detected in one case. Source regions varied from the Arctic Ocean and Greenland through to northern Russia and the European continent. Good agreement between the back trajectories was mirrored by comparable compositional trends between samples. Silicate dusts were identified in all cases, and the elemental composition of the dust was consistent for all samples except one. It is hypothesised that long-range, high-altitude transport was primarily responsible for this dust, with likely sources including the Asian arid regions.

Transport of Alaskan Dust into the Gulf of Alaska and Comparison with Similar High-Latitude Dust Environments

NASA Technical Reports Server (NTRS)

Crusium, John; Levy, Rob; Wang, Jun; Campbell, Rob; Schroth, Andrew W.

2012-01-01

Transport of Alaskan dust into the Gulf of Alaska and comparison with similar high-latitude dust environments. An airborne flux of the micronutrient iron, derived from dust originating from coastal regions may be an important contributor of iron to the Gulf of Alaska's (GoA) oligotrophic waters. Dust blowing off glacier termini and dry riverbeds is a recurring phenomenon in Alaska, usually occurring in the autumn. Since previous studies assumed that dust originating in the deserts of Asia was the largest source of . airborne iron to the GoA, the budget of aeolian deposition of iron needs to be reassessed. Since late 20 I 0, our group has been monitoring dust activity using satellites over the Copper River Delta (CRD) where the most vigorous dust plumes have been observed. Since 2011, sample aerosol concentration and their composition are being collected at Middleton Island (100km off shore of CRD). This presentation will show a summary of the ongoing dust observations and compare with other similar environments (Patagonia, Iceland) by showing case studies. Common features will be highlighted

April 2008 Saharan dust event: Its contribution to PM10 concentrations over the Anatolian Peninsula and relation with synoptic conditions.

PubMed

Kabatas, B; Pierce, R B; Unal, A; Rogal, M J; Lenzen, A

2018-08-15

An online-coupled regional Weather Research and Forecasting model with chemistry (WRF-Chem) is utilized incorporating 0.1°×0.1° spatial resolution HTAP (Hemispheric Transport of Air Pollution) anthropogenic emissions to investigate the spatial and temporal distribution of a Saharan dust outbreak, which contributed to high levels (>50μg/m 3 ) of daily PM 10 concentrations over Turkey in April 2008. Aerosol optical depth and cloud optical thickness retrievals from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor on board of Aqua satellite are used to better analyze the synoptic conditions that generated the dust outbreak in April 2008. A "Sharav" low pressure system, which transports the dust from Saharan source region over Turkey along the cold front, tends to move faster in WRF-Chem simulations than observed. This causes the predicted dust event to arrive earlier than observed leading to an overestimation of surface PM 10 concentrations in WRF-Chem simulation at the beginning of the event. Copyright © 2017 The Authors. Published by Elsevier B.V. All rights reserved.

Measuring Dust Emission from the Mojave Desert (USA) by Daily Remote-Camera Observations and Wind-Erosion Measurements: Bearing on "Unseen" Sources and Global Dust Abundance

NASA Astrophysics Data System (ADS)

Reynolds, R. L.; Urban, F.; Goldstein, H. L.; Fulton, R.

2017-12-01

A large gap in understanding the effects of atmospheric dust at all spatial scales is uncertainty about how much and whence dust is emitted annually. Digital recording of dust emission at high spatial and temporal resolution would, together with periodic flux measurements, support improved estimates of local-scale dust flux where infrastructure could support remote internet enabled cameras. Such recording would also elucidate wind-erosion dynamics when combined with meteorological data. Remote camera recording of dust-emitting settings on and around Soda Lake (Mojave Desert) was conducted every 15 minutes during daylight between 10 Nov. 2010 and 31 Dec. 2016 and images uploaded to a web server. Examination of 135,000 images revealed frequent dust events, termed "dust days" when plumes obscured mountains beyond source areas. Such days averaged 68 (sd=10) per year (2011 through 2016). We examined satellite retrievals (MODIS, GOES) for dust events during six cloudless days of highest and longest duration dust emission but none were observed. From Apr. 2000 through May 2013, aeolian sediments collected at three sites were sampled and weighed. Estimates of the emitted mass of silt- and clay-size fractions were made on the basis of measured horizontal mass flux, particle sizes of sediment in collectors, and roughly determined areas of dust generation. Over this period, nearly 4 Tg yr-1 of dust (as particulate matter <63 micrometers) were emitted across the study area. Much higher rates (about 7 Tg yr-1) were estimated for a subset period from Jan. 2011 through May 2013 following a major Mojave River flood in the basin in late Dec. 2010 that deposited flood sediment across the lake basin. Increased emission was likely related to the availability of fresh, unanchored flood sediment. Within the Mojave and Great Basin deserts of North America, many settings akin to those at Soda Lake similarly emit dust that is rarely detected in satellite retrievals. These findings strongly imply that local and regional dust emissions from western North America are far underestimated and that, by extension to relatively small dust-source areas across all drylands, global dust emissions may also be underestimated.

The multiple infrared source GL 437

NASA Technical Reports Server (NTRS)

Wynn-Williams, C. G.; Becklin, E. E.; Beichman, C. A.; Capps, R.; Shakeshaft, J. R.

1981-01-01

Infrared and radio continuum observations of the multiple infrared source GL 437 show that it consists of a compact H II region plus two objects which are probably early B stars undergoing rapid mass loss. The group of sources appears to be a multiple system of young stars that have recently emerged from the near side of a molecular cloud. Emission in the unidentified 3.3 micron feature is associated with, but more extended than, the emission from the compact H II region; it probably arises from hot dust grains at the interface between the H II region and the molecular cloud.

Airborne dust absorption by semi-arid forests reduces PM pollution in nearby urban environments.

PubMed

Uni, Daphna; Katra, Itzhak

2017-11-15

Dust storms are a major source of global atmospheric particulate matter (PM), having significant impacts on air pollution and human health. During dust storms, daily averages of atmospheric PM concentrations can reach high levels above the World Health Organization (WHO) guideline for air quality. The objective of this study was to explore the impact of forests on PM distribution following dust events in a region that is subjected to frequent dust storms (Northern Negev, Israel). Dust was measured in a forest transect including urban environments that are nearby the forest and at a distal location. During a background period, without dust events, the forest with its surrounding areas were characterized by lower monthly average of PM concentrations (38μg/m 3 ) compared with areas that are not affected by the forest (54μg/m 3 ). Such difference can be meaningful for long-term human health exposure. A reduction in PM levels in the forest transect was evident at most measured dust events, depending on the storm intensity and the locations of the protected areas. A significant reduction in PM 2.5 /PM 10 during dust events, indicates the high efficiency of the forest trees to absorb airborne PM 2.5 . Analysis of dust particles absorbed on the foliage revealed a total dust deposits of 8.1-9.2g/m 2 , which is equal to a minimum of 418.2tons removed from the atmosphere per a forest foliage area (30km 2 ). The findings can support environmental strategies to enhance life quality in regions that are subjected to dust storms, or under potential risk of dust-related PM due to land use and/or climate changes. Copyright © 2017 Elsevier B.V. All rights reserved.

Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing During Boreal Spring

NASA Technical Reports Server (NTRS)

Kim, Maeng-Ki; Lau, K. M.; Chin, Mian; Kim, Kyu-Myong; Sud, Y. C.; Walker, Greg K.

2005-01-01

The direct effects of aerosols on global and regional climate during boreal spring are investigated based on simulations using the NASA Global Modeling and Assimilation Office (GMAO) finite-volume general circulation model (fvGCM) with Microphyics of clouds in Relaxed Arakawa Schubert Scheme (McRAS). The aerosol loading are prescribed from three-dimensional monthly distribution of tropospheric aerosols viz., sulfate, black carbon, organic carbon, soil dust, and sea salt from output of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol extinction coefficient, single scattering albedo, and asymmetric factor are computed as wavelength-dependent radiative forcing in the radiative transfer scheme of the fvGCM, and as a function of the aerosol loading and ambient relative humidity. We find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excites a planetary scale teleconnection pattern in sea level pressure, temperature and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, i.e., South Asia, East Asia, and northern and western Africa. Additionally, atmospheric heating is found in regions with large loading of dust (over Northern Africa, and Middle East), and black carbon (over South-East Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east-west dipole anomaly with strong cooling over the Caspian Sea, and warming over central and northeastern Asia, where aerosol concentration are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes associated with the regional circulations.

General Circulation Model Simulations of the Annual Cycle of Martian Climate

NASA Astrophysics Data System (ADS)

Wilson, R.; Richardson, M.; Rodin, A.

Observations of the martian atmosphere have revealed a strong annual modulation of global mean atmospheric temperature that has been attributed to the pronounced seasonal asymmetry in solar radiation and the highly variable distribution of aerosol. These observations indicate little interannual variability during the relatively cool aphelion season and considerable variability in the perihelion season that is associated with the episodic occurrence of regional and major dust storms. The atmospheric circulation responds to the evolving spatial distribution of aerosol-induced heating and, in turn, plays a major role in determining the sources, sinks, and transport of radiatively active aerosol. We will present simulations employing the GFDL Mars General Circulation Model (MGCM) that show that aspects of the seasonally evolving climate may be simulated in a self-consistent manner using simple dust source parameterizations that represent the effects of lifting associated with local dust storms, dust devil activity, and other processes. Aerosol transport is accomplished, in large part, by elements of the large-scale circulation such as the Hadley circulation, baroclinic storms, tides, etc. A seasonal cycle of atmospheric opacity and temperature results from the variation in the strength and distribution of dust sources as well as from seasonal variations in the efficiency of atmospheric transport associated with changes in the circulation between solstice and equinox, and between perihelion and aphelion. We examine the efficiency of atmospheric transport of dust lifted along the perimeter of the polar caps to gauge the influence of these storms on the global circulation. We also consider the influence of water, as the formation of water ice clouds on dust nuclei may also affect the vertical distribution of dust and strongly influence the aerosol radiative properties.

Thorium distributions in high- and low-dust regions and the significance for iron supply

NASA Astrophysics Data System (ADS)

Hayes, Christopher T.; Rosen, Jeffrey; McGee, David; Boyle, Edward A.

2017-02-01

Thorium and uranium isotopes (232Th, 230Th, 238U, and 234U) were investigated to refine their use for estimating mineral dust deposition and Fe delivery to the ocean. U concentrations and isotope ratios were consistent with conservative behavior and can safely be described using published U-salinity relationships and global average seawater isotopic composition. Near Barbados, waters affected by the Amazon outflow contained elevated 232Th. This signals one region where the thorium-dust method is inaccurate because of a confounding continental input. Dissolved 232Th fluxes in this region suggest that Amazonian Fe supply to the adjacent open ocean is much larger than local atmospheric deposition. The colloidal content of dissolved Th south of Bermuda was found to be quite small (2-6%), similar to that found north of Hawaii, despite the order of magnitude higher dust deposition in the Atlantic. This finding supports the assumption that dissolved 232Th and 230Th are scavenged at the same rate despite their different sources and also sheds light on the increase of dissolved 232Th fluxes with integrated depth. Outside the region influenced by Amazon River waters, dissolved 232Th fluxes are compared with Bermudan aerosol Fe deposition to estimate that fractional Th solubility is around 20% in this region. Finally, new dissolved and soluble Fe, Mn, and Cr data from the subtropical North Pacific support the idea that Fe concentrations in the remote ocean are highly buffered, whereas 232Th has a larger dynamic range between high- and low-dust regions.

Airborne Petcoke Dust is a Major Source of Polycyclic Aromatic Hydrocarbons in the Athabasca Oil Sands Region.

PubMed

Zhang, Yifeng; Shotyk, William; Zaccone, Claudio; Noernberg, Tommy; Pelletier, Rick; Bicalho, Beatriz; Froese, Duane G; Davies, Lauren; Martin, Jonathan W

2016-02-16

Oil sands mining has been linked to increasing atmospheric deposition of polycyclic aromatic hydrocarbons (PAHs) in the Athabasca oil sands region (AOSR), but known sources cannot explain the quantity of PAHs in environmental samples. PAHs were measured in living Sphagnum moss (24 sites, n = 68), in sectioned peat cores (4 sites, n = 161), and snow (7 sites, n = 19) from ombrotrophic bogs in the AOSR. Prospective source samples were also analyzed, including petroleum coke (petcoke, from both delayed and fluid coking), fine tailings, oil sands ore, and naturally exposed bitumen. Average PAH concentrations in near-field moss (199 ng/g, n = 11) were significantly higher (p = 0.035) than in far-field moss (118 ng/g, n = 13), and increasing temporal trends were detected in three peat cores collected closest to industrial activity. A chemical mass-balance model estimated that delayed petcoke was the major source of PAHs to living moss, and among three peat core the contribution to PAHs from delayed petcoke increased over time, accounting for 45-95% of PAHs in contemporary layers. Petcoke was also estimated to be a major source of vanadium, nickel, and molybdenum. Scanning electron microscopy with energy-dispersive X-ray spectroscopy confirmed large petcoke particles (>10 μm) in snow at near-field sites. Petcoke dust has not previously been considered in environmental impact assessments of oil sands upgrading, and improved dust control from growing stockpiles may mitigate future risks.

Evaluation of two empirical wind erosion models in arid and semi-arid regions of China and the USA

USDA-ARS?s Scientific Manuscript database

The Tarim Basin in China and Columbia Plateau in the USA are important agricultural regions as well as source regions of windblown dust that impact air quality in Asia and North America. Wind erosion models are important tools for assessing the potential erodibility of soils and best management prac...

Water Cycling in the North Polar Region of Mars

NASA Technical Reports Server (NTRS)

Tamppari, L. K.; Smith, M. D.; Bass, D. S.

2003-01-01

To date, there has been no comprehensive study to understand the partitioning of water into vapor and ice clouds, and the associated effects of dust and surface temperature in the north polar region. Ascertaining the degree to which water is transported out of the cap region versus within the cap region will give much needed insight into the overall story of water cycling on a seasonal basis. In particular, understanding the mechanism for the polar cap surface albedo changes would go along way in comprehending the sources and sinks of water in the northern polar region. We approach this problem by examining Thermal Emission Spectrometer (TES) atmospheric and surface data acquired in the northern summer season and comparing it to Viking data when possible. Because the TES instrument spans the absorption bands of water vapor, water ice, dust, and measures surface temperature, all three aerosols and surface temperature can be retrieved simultaneously. This presentation will show our latest results on the water vapor, water-ice clouds seasonal and spatial distributions, as well as surface temperatures and dust distribution which may lend insight into where the water is going.

Revealing the Galactic Center in the Far-Infrared with SOFIA/FORCAST

NASA Astrophysics Data System (ADS)

Lau, Ryan M.; Herter, Terry; Morris, Mark; Li, Zhiyuan; Becklin, Eric; Adams, Joseph; Hankins, Matthew

2015-08-01

We present a summary of far-infrared imaging observations of the inner 40 pc of the Galactic center addressing the dense, dusty torus around Sgr A*, massive star formation, and dust production around massive stars and in the Sgr A East supernova remnant. Observations of warm dust emission were performed using the Faint Object Infrared Camera for the SOFIA Telescope (FORCAST). The Circumnuclear Ring (CNR) surrounding and heated by central cluster in the vicinity of Sgr A* shows no internal active star formation but does exhibit significant density “clumps,” a surprising result because tidal shearing should act quickly to smear out structure. G-0.02-0.07, a complex consisting of three compact HII regions and one ultracompact HII region, is site of the most recent confirmed star formation within ~10 pc of the Galactic center. Our observations reveal the dust morphologies and SEDs of the regions to constrain the composition and gas-to-dust mass ratios of the emitting dust and identify heating sources candidates from archival near-IR images. FORCAST observations Luminous Blue Variables (LBVs) located in and near the Quintuplet Cluster reveal the asymmetric, compressed shell of hot dust surrounding the Pistol Star and provide the first detection of the thermal emission from the symmetric, hot dust envelope surrounding G0.120-0.048. These two LBV’s have nebulae with similar quantities of dust (~0.02 M⊙) but exhibit contrasting appearances due to the external influence of their different environments. Finally, the far-infrared observations indicate the presence of ~0.02 M⊙ of warm (~100 K) dust in the hot interior of the ~10,000 yr-old SgrA East supernova remnant indicating the dust has survived the passage of the reverse shock. The results suggest that supernovae may indeed be the dominant dust production mechanism in the dense environment of early Universe galaxies.

Loess origin, transport, and deposition over the past 10,000 years, Wrangell-St. Elias National Park, Alaska

USGS Publications Warehouse

Muhs, Daniel R.; Budahn, James R.; McGeehin, John P.; Bettis, E. Arthur; Skipp, Gary L.; Paces, James B.; Wheeler, Elisabeth A.

2013-01-01

Contemporary glaciogenic dust has not received much attention, because most research has been on glaciogenic dust of the last glacial period or non-glaciogenic dust of the present interglacial period. Nevertheless, dust from modern glaciogenic sources may be important for Fe inputs to primary producers in the ocean. Adjacent to the subarctic Pacific Ocean, we studied a loess section near Chitina, Alaska along the Copper River in Wrangell-St. Elias National Park, where dust has been accumulating over the past ∼10,000 years. Mass accumulation rates for the fine-grained (<20 μm) fraction of this loess section are among the highest reported for the Holocene of high-latitude regions of the Northern Hemisphere. Based on mineralogy and geochemistry, loess at Chitina is derived from glacial sources in the Wrangell Mountains, the Chugach Mountains, and probably the Alaska Range. Concentrations of Fe in the silt-plus-clay fraction of the loess at Chitina are much higher than in all other loess bodies in North America and higher than most loess bodies on other continents. The very fine-grained (<2 μm) portion of this sediment, capable of long-range transport, is dominated by Fe-rich chlorite, which can yield Fe readily to primary producers in the ocean. Examination of satellite imagery shows that dust from the Copper River is transported by wind on a regular basis to the North Pacific Ocean. This Alaskan example shows that high-latitude glaciogenic dust needs to be considered as a significant Fe source to primary producers in the open ocean.

Interannual Variability in Global Dust Storm Initiation on Mars from a GCM with Orbit-Spin Coupling and Active Dust Lifting

NASA Astrophysics Data System (ADS)

Mischna, M.; Shirley, J. H.; Newman, C. E.

2016-12-01

To first order, the occurrence and interannual variability of global dust storms (GDS) on Mars is attributable to two factors: the annual cycle of solar insolation (which delineates a specific `dust storm season'), and the changing spatial distribution and availability of dust at the surface. Recent work has now found a remarkable correspondence between the occurrence of GDS on Mars and years in which the orbital angular momentum of Mars is increasing during the dust storm season. A previously undefined acceleration term `couples' this orbital motion to the rotational motion of the planet and atmosphere, and small but persistent atmospheric accelerations (so-called `coupling term accelerations,' or CTA) change the atmospheric circulation in such a way as to seemingly be favorable to storm development. This becomes a third factor, then, that may regulate the occurrence and variability of GDS. Our prior work with the MarsWRF general circulation model (GCM) was performed either with no atmospheric dust, or with simplified, prescribed dust distributions, and illustrated the dual roles of both insolation and CTA on GDS variability. Recent advances in the MarsWRF GCM dust prescription can now tackle the remaining unaddressed factor: the role of dust availability in controlling the initiation of GDS. Simulations with both infinite and finite global sources of dust have been performed. For a prescribed dust lifting threshold, surface dust is removed from the surface, preferentially from locations with larger surface stress values, transported in the atmosphere and deposited at a later time. Compared to simulations without CTA, those with CTA show more realism in the variability of timing and magnitude of atmospheric dustiness during the dust storm season. For infinite surface dust, the primary dust lifting (peak wind stress) regions are spatially restricted, and year-to-year changes are largely due to variations in the CTA at these few locations. By contrast, in simulations with finite surface dust, the peak stress regions are rapidly exhausted, leading to a far greater distribution of primary dust lifting regions; hence, variations in the CTA over a wider area contribute to the interannual variability of GDS. Results from our suite of simulations will be shown, vis-à-vis the historical record of GDS on Mars.

Planck intermediate results. XIX. An overview of the polarized thermal emission from Galactic dust

NASA Astrophysics Data System (ADS)

Planck Collaboration; Ade, P. A. R.; Aghanim, N.; Alina, D.; Alves, M. I. R.; Armitage-Caplan, C.; Arnaud, M.; Arzoumanian, D.; Ashdown, M.; Atrio-Barandela, F.; Aumont, J.; Baccigalupi, C.; Banday, A. J.; Barreiro, R. B.; Battaner, E.; Benabed, K.; Benoit-Lévy, A.; Bernard, J.-P.; Bersanelli, M.; Bielewicz, P.; Bock, J. J.; Bond, J. R.; Borrill, J.; Bouchet, F. R.; Boulanger, F.; Bracco, A.; Burigana, C.; Butler, R. C.; Cardoso, J.-F.; Catalano, A.; Chamballu, A.; Chary, R.-R.; Chiang, H. C.; Christensen, P. R.; Colombi, S.; Colombo, L. P. L.; Combet, C.; Couchot, F.; Coulais, A.; Crill, B. P.; Curto, A.; Cuttaia, F.; Danese, L.; Davies, R. D.; Davis, R. J.; de Bernardis, P.; de Gouveia Dal Pino, E. M.; de Rosa, A.; de Zotti, G.; Delabrouille, J.; Désert, F.-X.; Dickinson, C.; Diego, J. M.; Donzelli, S.; Doré, O.; Douspis, M.; Dunkley, J.; Dupac, X.; Efstathiou, G.; Enßlin, T. A.; Eriksen, H. K.; Falgarone, E.; Ferrière, K.; Finelli, F.; Forni, O.; Frailis, M.; Fraisse, A. A.; Franceschi, E.; Galeotta, S.; Ganga, K.; Ghosh, T.; Giard, M.; Giraud-Héraud, Y.; González-Nuevo, J.; Górski, K. M.; Gregorio, A.; Gruppuso, A.; Guillet, V.; Hansen, F. K.; Harrison, D. L.; Helou, G.; Hernández-Monteagudo, C.; Hildebrandt, S. R.; Hivon, E.; Hobson, M.; Holmes, W. A.; Hornstrup, A.; Huffenberger, K. M.; Jaffe, A. H.; Jaffe, T. R.; Jones, W. C.; Juvela, M.; Keihänen, E.; Keskitalo, R.; Kisner, T. S.; Kneissl, R.; Knoche, J.; Kunz, M.; Kurki-Suonio, H.; Lagache, G.; Lähteenmäki, A.; Lamarre, J.-M.; Lasenby, A.; Lawrence, C. R.; Leahy, J. P.; Leonardi, R.; Levrier, F.; Liguori, M.; Lilje, P. B.; Linden-Vørnle, M.; López-Caniego, M.; Lubin, P. M.; Macías-Pérez, J. F.; Maffei, B.; Magalhães, A. M.; Maino, D.; Mandolesi, N.; Maris, M.; Marshall, D. J.; Martin, P. G.; Martínez-González, E.; Masi, S.; Matarrese, S.; Mazzotta, P.; Melchiorri, A.; Mendes, L.; Mennella, A.; Migliaccio, M.; Miville-Deschênes, M.-A.; Moneti, A.; Montier, L.; Morgante, G.; Mortlock, D.; Munshi, D.; Murphy, J. A.; Naselsky, P.; Nati, F.; Natoli, P.; Netterfield, C. B.; Noviello, F.; Novikov, D.; Novikov, I.; Oxborrow, C. A.; Pagano, L.; Pajot, F.; Paladini, R.; Paoletti, D.; Pasian, F.; Pearson, T. J.; Perdereau, O.; Perotto, L.; Perrotta, F.; Piacentini, F.; Piat, M.; Pietrobon, D.; Plaszczynski, S.; Poidevin, F.; Pointecouteau, E.; Polenta, G.; Popa, L.; Pratt, G. W.; Prunet, S.; Puget, J.-L.; Rachen, J. P.; Reach, W. T.; Rebolo, R.; Reinecke, M.; Remazeilles, M.; Renault, C.; Ricciardi, S.; Riller, T.; Ristorcelli, I.; Rocha, G.; Rosset, C.; Roudier, G.; Rubiño-Martín, J. A.; Rusholme, B.; Sandri, M.; Savini, G.; Scott, D.; Spencer, L. D.; Stolyarov, V.; Stompor, R.; Sudiwala, R.; Sutton, D.; Suur-Uski, A.-S.; Sygnet, J.-F.; Tauber, J. A.; Terenzi, L.; Toffolatti, L.; Tomasi, M.; Tristram, M.; Tucci, M.; Umana, G.; Valenziano, L.; Valiviita, J.; Van Tent, B.; Vielva, P.; Villa, F.; Wade, L. A.; Wandelt, B. D.; Zacchei, A.; Zonca, A.

2015-04-01

This paper presents an overview of the polarized sky as seen by Planck HFI at 353 GHz, which is the most sensitive Planck channel for dust polarization. We construct and analyse maps of dust polarization fraction and polarization angle at 1° resolution, taking into account noise bias and possible systematic effects. The sensitivity of the Planck HFI polarization measurements allows for the first time a mapping of Galactic dust polarized emission on large scales, including low column density regions. We find that the maximum observed dust polarization fraction is high (pmax = 19.8%), in particular in some regions of moderate hydrogen column density (NH < 2 × 1021 cm-2). The polarization fraction displays a large scatter at NH below a few 1021 cm-2. There is a general decrease in the dust polarization fraction with increasing column density above NH ≃ 1 × 1021 cm-2 and in particular a sharp drop above NH ≃ 1.5 × 1022 cm-2. We characterize the spatial structure of the polarization angle using the angle dispersion function. We find that the polarization angle is ordered over extended areas of several square degrees, separated by filamentary structures of high angle dispersion function. These appear as interfaces where the sky projection of the magnetic field changes abruptly without variations in the column density. The polarization fraction is found to be anti-correlated with the dispersion of polarization angles. These results suggest that, at the resolution of 1°, depolarization is due mainly to fluctuations in the magnetic field orientation along the line of sight, rather than to the loss of grain alignment in shielded regions. We also compare the polarization of thermal dust emission with that of synchrotron measured with Planck, low-frequency radio data, and Faraday rotation measurements toward extragalactic sources. These components bear resemblance along the Galactic plane and in some regions such as the Fan and North Polar Spur regions. The poor match observed in other regions shows, however, that dust, cosmic-ray electrons, and thermal electrons generally sample different parts of the line of sight. Appendices are available in electronic form at http://www.aanda.org

Effects of interstellar dust scattering on the X-ray eclipses of the LMXB AX J1745.6-2901 in the Galactic Centre

NASA Astrophysics Data System (ADS)

Jin, Chichuan; Ponti, Gabriele; Haberl, Frank; Smith, Randall; Valencic, Lynne

2018-07-01

AX J1745.6-2901 is an eclipsing low-mass X-ray binary in the Galactic Centre (GC). It shows significant X-ray excess emission during the eclipse phase, and its eclipse light curve shows an asymmetric shape. We use archival XMM-Newton and Chandra observations to study the origin of these peculiar X-ray eclipsing phenomena. We find that the shape of the observed X-ray eclipse light curves depends on both photon energy and the shape of the source extraction region, and also shows differences between the two instruments. By performing detailed simulations for the time-dependent X-ray dust-scattering halo, as well as directly modelling the observed eclipse and non-eclipse halo profiles of AX J1745.6-2901, we obtained solid evidence that its peculiar eclipse phenomena are indeed caused by the X-ray dust scattering in multiple foreground dust layers along the line of sight (LOS). The apparent dependence on the instruments is caused by different instrumental point spread functions. Our results can be used to assess the influence of dust-scattering in other eclipsing X-ray sources, and raise the importance of considering the timing effects of dust-scattering halo when studying the variability of other X-ray sources in the GC, such as Sgr A⋆. Moreover, our study of halo eclipse reinforces the existence of a dust layer local to AX J1745.6-2901 as reported by Jin et al. (2017), as well as identifying another dust layer within a few hundred parsecs to the Earth, containing up to several tens of percent LOS dust, which is likely to be associated with the molecular clouds in the Solar neighbourhood. The remaining LOS dust is likely to be associated with the molecular clouds located in the Galactic disc in-between.

Optical and microphysical properties of natural mineral dust and anthropogenic soil dust near dust source regions over northwestern China

NASA Astrophysics Data System (ADS)

Wang, Xin; Wen, Hui; Shi, Jinsen; Bi, Jianrong; Huang, Zhongwei; Zhang, Beidou; Zhou, Tian; Fu, Kaiqi; Chen, Quanliang; Xin, Jinyuan

2018-02-01

Mineral dust aerosols (MDs) not only influence the climate by scattering and absorbing solar radiation but also modify cloud properties and change the ecosystem. From 3 April to 16 May 2014, a ground-based mobile laboratory was deployed to measure the optical and microphysical properties of MDs near dust source regions in Wuwei, Zhangye, and Dunhuang (in chronological order) along the Hexi Corridor over northwestern China. Throughout this dust campaign, the hourly averaged (±standard deviation) aerosol scattering coefficients (σsp, 550 nm) of the particulates with aerodynamic diameters less than 2.5 µm (PM2.5) at these three sites were sequentially 101.5 ± 36.8, 182.2 ± 433.1, and 54.0 ± 32.0 Mm-1. Correspondingly, the absorption coefficients (σap, 637 nm) were 9.7 ± 6.1, 6.0 ± 4.6, and 2.3 ± 0.9 Mm-1; single-scattering albedos (ω, 637 nm) were 0.902 ± 0.025, 0.931 ± 0.037, and 0.949 ± 0.020; and scattering Ångström exponents (Åsp, 450-700 nm) of PM2.5 were 1.28 ± 0.27, 0.77 ± 0.51, and 0.52 ± 0.31. During a severe dust storm in Zhangye (i.e., from 23 to 25 April), the highest values of σsp2.5 ( ˜ 5074 Mm-1), backscattering coefficient (σbsp2.5, ˜ 522 Mm-1), and ω637 ( ˜ 0.993) and the lowest values of backscattering fraction (b2.5, ˜ 0.101) at 550 nm and Åsp2.5 ( ˜ -0.046) at 450-700 nm, with peak values of aerosol number size distribution (appearing at the particle diameter range of 1-3 µm), exhibited that the atmospheric aerosols were dominated by coarse-mode dust aerosols. It is hypothesized that the relatively higher values of mass scattering efficiency during floating dust episodes in Wuwei and Zhangye are attributed to the anthropogenic soil dust produced by agricultural cultivations.

NMMB/BSC-DUST: an online mineral dust atmospheric model from meso to global scales

NASA Astrophysics Data System (ADS)

Haustein, K.; Pérez, C.; Jorba, O.; Baldasano, J. M.; Janjic, Z.; Black, T.; Nickovic, S.

2009-04-01

While mineral dust distribution and effects are important at global scales, they strongly depend on dust emissions that are controlled on small spatial and temporal scales. Most global dust models use prescribed wind fields provided by meteorological centers (e.g., NCEP and ECMWF) and their spatial resolution is currently never better than about 1°×1°. Regional dust models offer substantially higher resolution (10-20 km) and are typically coupled with weather forecast models that simulate processes that GCMs either cannot resolve or can resolve only poorly. These include internal circulation features such as the low-level nocturnal jet which is a crucial feature for dust emission in several dust ‘hot spot' sources in North Africa. Based on our modeling experience with the BSC-DREAM regional forecast model (http://www.bsc.es/projects/earthscience/DREAM/) we are currently implementing an improved mineral dust model [Pérez et al., 2008] coupled online with the new global/regional NMMB atmospheric model under development in NOAA/NCEP/EMC [Janjic, 2005]. The NMMB is an evolution of the operational WRF-NMME extending from meso to global scales. The NMMB will become the next-generation NCEP model for operational weather forecast in 2010. The corresponding unified non-hydrostatic dynamical core ranges from meso to global scale allowing regional and global simulations. It has got an add-on non-hydrostatic module and it is based on the Arakawa B-grid and hybrid pressure-sigma vertical coordinates. NMMB is fully embedded into the Earth System Modeling Framework (ESMF), treating dynamics and physics separately and coupling them easily within the ESMF structure. Our main goal is to provide global dust forecasts up to 7 days at mesoscale resolutions. New features of the model include a physically-based dust emission scheme after White [1979], Iversen and White [1982] and Marticorena and Bergametti [1995] that takes the effects of saltation and sandblasting into account. Viscous sublayer approach [Janjic, 1994] for dust injection in the lower atmosphere is maintained as applied in DREAM [Nickovic et al., 2001]. Soil moisture effects are considered following Fecan et al. [1999]. A new source function for the land surface is calculated using the USGS 1km landuse database, the NESDIS 5-years monthly climatology for the vegetation fraction, and preferential source areas according the topographic approach after Ginoux et al. [2001]. Furthermore, 4 top soil texture classes (coarse sand, fine/medium sand, silt, clay) are introduced, based on the new STASGO-FAO 1km soil database and modified following Tegen et al. [2002]. The dry deposition scheme accounts for the effects of sedimentation and turbulent mixout following the approach of Giorgi [1986]. Finally, in-cloud and below-cloud wet scavenging for grid-scale and convective precipitation is applied following Slinn [1983; 1984] and Loosmore and Cederwall [2004]. Dust radiative feedback on meteorology is not yet considered. In order to explore the assets and drawbacks of the new model, we perform global simulations of the dust cycle at 0.3°x0.45° to demonstrate the ability of the model to capture the large scale and seasonal patterns. These fundamental evaluations serve as starting point for further testing as well as future developments of the NMMb-DUST. In a second step, we study the behavior of the model during the SAMUM-I phase [Haustein et al., 2009] and the BODEX campaign [Todd et al., 2008], focusing on how the model reproduces moist convection and low level jet in North Africa at mesoscale resolutions. References: Fecan, F., B. Marticorena and G. Bergametti. (1999). Parameterization of the increase of the aeolian erosion threshold wind friction velocity due to soil moisture for arid and semi arid areas. Annales Geophysicae, 17, 149-157. Ginoux, P. et al. (2001). Sources and distribution of dust aerosols simulated with the GOCART model. J. Geophys. Res., 106, D17, 20255-20273. Giorgi, F. (1986). A particle dry-deposition parameterization scheme for use in tracer transport models. J. Geophys. Res., 91, 9794-9804. Haustein, K. et al. (2009). Regional dust model performance during SAMUM-I 2006. Geophys. Res. Letters, in press. Iversen, J.D. and B. R. White (1982). Saltation threshold on Earth, Mars and Venus. Sedimentology, 29, 111-119. Janjic, Z. I. (1994). The Step-Mountain Eta Coordinate Model: Further Developments of the Convection, Viscous Sublayer, and Turbulence Closure Schemes. Monthly Weather Review, 122, 927-945. Janjic, Z. I. (2005). A unified model approach from meso to global scales. Geophysical Research Abstracts, 7, 05582, 2005, EGU05-A-05582. Loosmore, G. A. and Cederwall, R. T. (2004). Precipitation scavenging of atmospheric aerosols for emergency response applications: testing an updated model with new real-time data. Atmospheric Environment, 38, 993-1003. Marticorena, B. and G. Bergametti (1995). Modeling the atmospheric dust cycle: 1. Design of a soil-derived dust emission scheme. J. Geophys. Res., 100, D8, 16415-16430. Nickovic, S., G. Kallos, A. Papadopoulos, and O. Kakaliagou (2001). A model for prediction of desert dust cycle in the atmosphere. Journal of Geophysical Research 106, D16, 18113-18129. Pérez, C. et al. (2008). An online mineral dust model within the global/regional NMMB: Current progress and plans. AGU Fall Meeting, 14-19 December 2008, San Francisco, USA. Slinn, W. G. N. (1983). A potpourri of deposition and resuspension questions. In: Pruppacher, Semonin and Slinn (Editors), Precip. Scavenging., Dry Deposition, and Resuspension. Elsevier, New York (1983), 1361-1416. Slinn, W.G.N. (1984). Precipitation scavenging. In: Randerson, D. (Editor), Atmospheric Science and Power Production. OSTI, Oak Ridge, 466-532. Tegen, I. et al. (2002). Impact of vegetation and preferential source areas on global dust aerosol: Results from a model study. J. Geophys. Res., 107, D21, doi:10.1029/2001JD000963. Todd, M. (2008). Quantifying uncertainty in estimates of mineral dust flux: An intercomparison of model performance over the Bodele Depression, northern Chad. J. Geophys. Res., 113, D24107, doi:10.1029/2008JD010476. White, B. (1979). Soil transport by winds on Mars. J. Geophys. Res., 84, 4643-4651.

Assimilation of MODIS Dark Target and Deep Blue Observations in the Dust Aerosol Component of NMMB-MONARCH version 1.0

NASA Technical Reports Server (NTRS)

Di Tomaso, Enza; Schutgens, Nick A. J.; Jorba, Oriol; Perez Garcia-Pando, Carlos

2017-01-01

A data assimilation capability has been built for the NMMB-MONARCH chemical weather prediction system, with a focus on mineral dust, a prominent type of aerosol. An ensemble-based Kalman filter technique (namely the local ensemble transform Kalman filter - LETKF) has been utilized to optimally combine model background and satellite retrievals. Our implementation of the ensemble is based on known uncertainties in the physical parametrizations of the dust emission scheme. Experiments showed that MODIS AOD retrievals using the Dark Target algorithm can help NMMB-MONARCH to better characterize atmospheric dust. This is particularly true for the analysis of the dust outflow in the Sahel region and over the African Atlantic coast. The assimilation of MODIS AOD retrievals based on the Deep Blue algorithm has a further positive impact in the analysis downwind from the strongest dust sources of the Sahara and in the Arabian Peninsula. An analysis-initialized forecast performs better (lower forecast error and higher correlation with observations) than a standard forecast, with the exception of underestimating dust in the long-range Atlantic transport and degradation of the temporal evolution of dust in some regions after day 1. Particularly relevant is the improved forecast over the Sahara throughout the forecast range thanks to the assimilation of Deep Blue retrievals over areas not easily covered by other observational datasets.The present study on mineral dust is a first step towards data assimilation with a complete aerosol prediction system that includes multiple aerosol species.

Assimilation of MODIS Dark Target and Deep Blue observations in the dust aerosol component of NMMB-MONARCH version 1.0

NASA Astrophysics Data System (ADS)

Di Tomaso, Enza; Schutgens, Nick A. J.; Jorba, Oriol; Pérez García-Pando, Carlos

2017-03-01

A data assimilation capability has been built for the NMMB-MONARCH chemical weather prediction system, with a focus on mineral dust, a prominent type of aerosol. An ensemble-based Kalman filter technique (namely the local ensemble transform Kalman filter - LETKF) has been utilized to optimally combine model background and satellite retrievals. Our implementation of the ensemble is based on known uncertainties in the physical parametrizations of the dust emission scheme. Experiments showed that MODIS AOD retrievals using the Dark Target algorithm can help NMMB-MONARCH to better characterize atmospheric dust. This is particularly true for the analysis of the dust outflow in the Sahel region and over the African Atlantic coast. The assimilation of MODIS AOD retrievals based on the Deep Blue algorithm has a further positive impact in the analysis downwind from the strongest dust sources of the Sahara and in the Arabian Peninsula. An analysis-initialized forecast performs better (lower forecast error and higher correlation with observations) than a standard forecast, with the exception of underestimating dust in the long-range Atlantic transport and degradation of the temporal evolution of dust in some regions after day 1. Particularly relevant is the improved forecast over the Sahara throughout the forecast range thanks to the assimilation of Deep Blue retrievals over areas not easily covered by other observational datasets. The present study on mineral dust is a first step towards data assimilation with a complete aerosol prediction system that includes multiple aerosol species.

Tracing anthropogenic aerosol Fe sources in the North Atlantic Ocean using dissolved Fe isotope ratios

NASA Astrophysics Data System (ADS)

Conway, T. M.; Shelley, R.; Aguilar-Islas, A. M.; Landing, W. M.; Mahowald, N. M.; John, S.

2016-02-01

Supply of iron (Fe) to the surface ocean from atmospheric deposition plays a vital role in marine biogeochemical cycles, especially in Fe-limited areas or regions close to dust sources. However, large uncertainties remain over the fluxes, solubility and bioavailability of Fe supplied by aerosol dust. Additionally, aerosol Fe is likely to consist of a mixture of natural and anthropogenic (urban, biomass burning and combustion) components, which may have very different solubilities in seawater [e.g. 1]. To constrain soluble Fe supply to the oceans, it is thus vitally important to understand the relative contributions of different types of aerosol Fe, their solubilities and spatial distributions. Stable Fe isotopes (δ56Fe) may offer a way to discriminate between different dust sources [2], because of differential fractionation during a range of chemical processes. In this study, we measured δ56Fe in North Atlantic marine aerosols collected during two US GEOTRACES GA03 cruises (Lisbon to Woods Hole via Cape Verde, 2010-11) and we present δ56Fe measurements (relative to IRMM-014) from both the bulk aerosol (HF-HNO3 digested) and the water-soluble (10s ultrapure water leach) fractions. Aerosols collected from different air-masses (Saharan, European and N. American) allowed us to investigate the variability in δ56Fe due to different regional dust sources. The bulk phase was characterized by near-crustal δ56Fe values of +0.1±0.2‰, indicating the dominance of mineral dust. In contrast, the water-soluble fraction showed great variability; aerosols from European and North American air-masses were very isotopically light (-1.2±0.2‰ and -1.1±0.7‰) while those from Saharan air-masses were crustal (+0.1‰). Comparison of this data with isotope-informed model predictions of soluble Fe from mineral and anthropogenic sources (combustion, biofuels and biomass burning) [1], suggests that the data is consistent with mixing of either 1) Fe from mineral dust (+0.1‰) and a distinctly light anthropogenic Fe (-1.6‰), or 2) Fe from crustal mineral dust, isotopically heavy combustion Fe (+0.1 to +0.3‰), and biomass Fe that is both isotopically light (-1.6‰) and very soluble (>50%). [1] Luo, C. et al. (2008), Glob. Biogeochem. Cyc., 22, GB1012. [2] Mead, C. et al. (2013), Geophys. Res. Lett., 40, 5722-5727.

Dust fluxes linked to intensification of Prevailing Westerlies and Trade Winds stimulated Ethmodiscus rex giant diatom blooms in the southern Mariana Trench, western tropical Pacific at onset of the Last Glacial Maximum

NASA Astrophysics Data System (ADS)

Chen, D.; Luo, M.; Algeo, T. J.; Chen, L.

2017-12-01

The strontium (Sr) and neodymium (Nd) isotope compositions and clay-mineral assemblages of the detrital fraction of sediments in the southern Mariana Trench together with major- and trace-elements concentrations of bulk sediments have been determined to trace the sediment provenance and investigate the relationship between Asian dust input and blooms of the giant diatom Ethmodiscus rex. Enrichment of barium (Ba) in relative to upper continental crust (UCC) and low average Rb/K ratios in all study cores point to both hydrothermal and volcaniclastic inputs to the sediments. Both the Sr-Nd isotope compositions and the clay-mineral assemblages of the detrital fraction reflect a two-component mixing system consisting of Mariana arc volcaniclastics and eolian Asian dust. A decrease in smectite content and an increase in illite content just before formation of laminated diatom mats (LDMs) suggest a change in the source of the eolian dust from eastern Asian deserts (EADs) to central Asian deserts (CADs) at the onset of the Last Glacial Maximum (LGM). This observation suggests a causal linkage between atmospheric circulation patterns, the sources of eolian Asian dust, and marine productivity in the western Pacific region. We postulate that the shift to CAD-sourced dust may have played a greater role in promoting biological productivity in the oligotrophic western Pacific Ocean during the LGM than previously realized.

Temporal dynamics of salt crust patterns on a sodic playa: implications for aerodynamic roughness and dust emission potential

NASA Astrophysics Data System (ADS)

Nield, Joanna; Bryant, Robert; Wiggs, Giles; King, James; Thomas, David; Eckardt, Frank; Washington, Richard

2015-04-01

Salt pans (or playas) are common in arid environments and can be major sources of windblown mineral dust, but there are uncertainties associated with their dust emission potential. These landforms typically form crusts which modify both their erosivity and erodibility by limiting sediment availability, modifying surface and aerodynamic roughness and limiting evaporation rates and sediment production. Here we show the relationship between seasonal surface moisture change and crust pattern development on part of the Makgadikgadi Pans of Botswana (a Southern Hemisphere playa that emits significant dust), based on both remote-sensing and field surface and atmospheric measurements. We use high resolution (sub-cm) terrestrial laser scanning (TLS) surveys over weekly, monthly and annual timescales to accurately characterise crustal ridge thrusting and collapse. Ridge development can change surface topography as much as 30 mm/week on fresh pan areas that have recently been reset by flooding. The corresponding change aerodynamic roughness can be as much as 3 mm/week. At the same time, crack densities across the surface increase and this raises the availability of erodible fluffy, low density dust source sediment stored below the crust layer. We present a conceptual model accounting for the driving forces (subsurface, surface and atmospheric moisture) and feedbacks between these and surface shape that lead to crust pattern trajectories between highly emissive degraded surfaces and less emissive ridged or continuous crusts. These findings improve our understanding of temporal changes in dust availability and supply from playa source regions.

A search for precursors of ultracompact H II regions in a sample of luminous IRAS sources. III. Circumstellar dust properties

NASA Technical Reports Server (NTRS)

Molinari, S.; Brand, J.; Cesaroni, R.; Palla, F.

2000-01-01

The James Clerk Maxwell Telescope has been used to obtain submillimeter and millimeter continuum photometry of a sample of 30 IRAS sources previously studied in molecular lines and centimeter radio continuum. All the sources have IRAS colours typical of very young stellar objects (YSOs) and are associated with dense gas.

The paleo-ocean characteristics of the Taklimakan dust aerosol: high sulfate from primary sources and implication for climate modeling

NASA Astrophysics Data System (ADS)

Huang, K.; Zhuang, G.; Fu, J. S.; Dong, X.

2017-12-01

Multi-year monitoring of dust aerosol from the Taklimakan Desert has been conducted at one site in the hinterland of the desert, Tazhong and another site at the southern edge of the desert, Hotan. Compared to the other two important desert source regions of China, i.e. Gobi and Loess Plateau, the Taklimakan Desert is characterized of high calcium with a Ca/Al elemental ratio of around 1.50. The unique feature of the Taklimakan dust aerosol is its abundant sulfate. For instance, the mean concentration of sulfate over Tazhong reached as high as 34.7 and 48.8 ug/m3 during the spring of 2007 and 2008, respectively. During the dust storm events, the daily concentration of sulfate frequently exceeded 100 ug/m3. Sulfate showed strong correlations with the primary aerosol species such as Ca2+, Mg2+, Na+, Cl-, Al, Fe, Ti, etc. but weakly correlated with the secondary aerosol species such as NO3- and NH4+. The mass ratio of sulfate in the total suspended particles showed a relatively stable percentage of around 2.5% regardless of the intensity of the dust events. In addition, individual particle analysis using the scanning electron microscope (SEM) technique found that gypsum (CaSO4) particles could account for 11.1% of total number of particles as well as abundant Na2SO4 and NaCl particles. All the evidences above suggested the high sulfate observed in the Taklimakan Desert were largely attributed to primary sources but not formed via the traditional gas-to-particle formation pathway. As the Taklimakan Desert was speculated to be ocean 5-7 million years, the dried sea salts from the paleo-ocean should be the major source of the dust aerosol. Also, the dried salt lakes in the northwestern China may contribute to the high sulfate. Based on two different methods, the contribution of primary sources to sulfate over the Taklimakan Desert is estimated to be around 43% - 82%. This study implied that the cooling effect of the Taklimakan dust aerosol could be underestimated if the explicit dust chemical composition is not considered for modeling.

Organic Components and Elemental Carbon in Soils and Ambient Particles near Phoenix, AZ

NASA Astrophysics Data System (ADS)

Fraser, M. P.; Jia, Y.; Clements, A.

2008-12-01

In the desert southwest, fugitive dust emissions contribute significantly to ambient aerosol concentrations. Wind erosion from the arid land is a primary contributor to ambient particulate matter (PM) concentrations but, in regions including Central Arizona, desert lands have been converted for agriculture use and thus agriculture processes constitute another contributor. As the metropolitan Phoenix region expands into these agricultural lands, urban sources and construction also contributes to the ambient PM load. In an effort to identify and access relative contribution of these and other major PM sources in the region, a series of ambient PM samples and soil samples were collected near Higley, AZ, a suburb of Phoenix which has seen rapid urbanization onto agricultural lands between January and May 2008. The soil samples collected were resuspended and samples of resuspended dust were collected to represent particles smaller than 2.5 microns and 10 microns in aerodynamic diameter (PM2.5 and PM10 respectively). The size segregated soil and ambient PM samples were analyzed for bulk mass, elemental and organic carbon content, and a number of specific compounds including ions, metals, alkanes, organic acids, polycyclic aromatic hydrocarbons, and saccharides. The saccharide contribution to soil organic carbon has been studied to elucidate key factors in the soil carbon balance and markers have been developed for tracing fungal metabolites, plant growth and budding and organic matter decay. Using organic markers, the contribution of various sources to PM10 and PM2.5 levels have been determined by positive matrix factorization (PMF) of the ambient aerosol marker concentrations quantified from PM samples. Subsequently, samples of local soil from native and agricultural fields and local roadways wers size- segregated and analyzed in an effort to create a source profile for the dust in the area. A chemical mass balance model has been used to compare with the PMF results where sampled and resuspended agricultural soil, native soil and road dusts are used to characterize direct emissions of these sources to ambient fine and coarse particulate matter.

Last Glacial loess in the conterminous USA

USGS Publications Warehouse

Bettis, E. Arthur; Muhs, Daniel R.; Roberts, Helen M.; Wintle, Ann G.

2003-01-01

The conterminous United States contains an extensive and generally well-studied record of Last Glacial loess. The loess occurs in diverse physiographic provinces, and under a wide range of climatic and ecological conditions. Both glacial and non-glacia lloess sources are present, and many properties of the loess vary systematically with distance from loess sources. United States' mid-continent Last Glacial loess is probably the thickest in the world, and our calculated mass accumulation rates (MARs) are as high as 17,500 g/m2/yr at the Bignell Hill locality in Nebraska, and many near-source localities have MARs greater than 1500 g/m2/yr. These MARs are high relative to rates calculated in other loess provinces around the world. Recent models of LastGlacial dust sources fail to predict the extent and magnitude of dust flux from the mid-continent of the United States. A better understanding of linkages between climate, ice sheet behaviour, routing of glacial meltwater, land surface processes beyond the ice margin, and vegetation is needed to improve the predictive capabilities of models simulating dust flux from this region.

Infrared emission spectra of candidate interstellar aromatic molecules

NASA Technical Reports Server (NTRS)

Schlemmer, S.; Balucani, N.; Wagner, D. R.; Steiner, B.; Saykally, R. J.

1996-01-01

Interstellar dust is responsible, through surface reactions, for the creation of molecular hydrogen, the main component of the interstellar clouds in which new stars form. Intermediate between small, gas-phase molecules and dust are the polycyclic aromatic hydrocarbons (PAHs). Such molecules could account for 2-30% of the carbon in the Galaxy, and may provide nucleation sites for the formation of carbonaceous dust. Although PAHs have been proposed as the sources of the unidentified infrared emission bands that are observed in the spectra of a variety of interstellar sources, the emission characteristics of such molecules are still poorly understood. Here we report laboratory emission spectra of several representative PAHs, obtained in conditions approximating those of the interstellar medium, and measured over the entire spectral region spanned by the unidentified infrared bands. We find that neutral PAHs of small and moderate size can at best make only a minor contribution to these emission bands. Cations of these molecules, as well as much larger PAHs and their cations, remain viable candidates for the sources of these bands.

Mixing of Dust and NH3 Observed Globally over Anthropogenic Dust Sources

NASA Technical Reports Server (NTRS)

Ginoux, P.; Clarisse, L.; Clerbaux, C.; Coheur, P.-F.; Dubovik, O.; Hsu, N. C.; Van Damme, M.

2012-01-01

The global distribution of dust column burden derived from MODIS Deep Blue aerosol products is compared to NH3 column burden retrieved from IASI infrared spectra. We found similarities in their spatial distributions, in particular their hot spots are often collocated over croplands and to a lesser extent pastures. Globally, we found 22% of dust burden collocated with NH3, with only 1% difference between land-use databases. This confirms the importance of anthropogenic dust from agriculture. Regionally, the Indian subcontinent has the highest amount of dust mixed with NH3 (26 %), mostly over cropland and during the pre-monsoon season. North Africa represents 50% of total dust burden but accounts for only 4% of mixed dust, which is found over croplands and pastures in Sahel and the coastal region of the Mediterranean. In order to evaluate the radiative effect of this mixing on dust optical properties, we derive the mass extinction efficiency for various mixtures of dust and NH3, using AERONET sunphotometers data. We found that for dusty days the coarse mode mass extinction efficiency decreases from 0.62 to 0.48 square meters per gram as NH3 burden increases from 0 to 40 milligrams per square meter. The fine mode extinction efficiency, ranging from 4 to 16 square mters per gram, does not appear to depend on NH3 concentration or relative humidity but rather on mineralogical composition and mixing with other aerosols. Our results imply that a significant amount of dust is already mixed with ammonium salt before its long range transport. This in turn will affect dust lifetime, and its interactions with radiation and cloud properties

[Preliminary study of source apportionment of PM10 and PM2.5 in three cities of China during spring].

PubMed

Gao, Shen; Pan, Xiao-chuan; Madaniyazi, Li-na; Xie, Juan; He, Ya-hui

2013-09-01

To study source apportionment of atmospheric PM10 (particle matter ≤ 10 µm in aerodynamic diameter) and PM2.5 (particle matter ≤ 2.5 µm in aerodynamic diameter) in Beijing,Urumqi and Qingdao, China. The atmospheric particle samples of PM10 and PM2.5 collected from Beijing between May 17th and June 18th, 2005, from Urumqi between April 20th and June 1st, 2006 and from Qingdao between April 4th and May 15th, 2005, were detected to trace the source apportionment by factor analysis and enrichment factor methods. In Beijing, the source apportionment results derived from factor analysis model for PM10 were construction dust and soil sand dust (contributing rate of variance at 45.35%), industry dust, coal-combusted smoke and vehicle emissions (contributing rate at 31.83%), and biomass burning dust (13.57%). The main pollution element was Pb, while the content (median (minimum value-maximum value)was 0.216 (0.040-0.795) µg/m(3)) . As for PM2.5, the sources were construction dust and soil sand dust (38.86%), industry dust, coal-combusted smoke and vehicle emissions (25.73%), biomass burning dust (13.10%) and burning oil dust (11.92%). The main pollution element was Zn (0.365(0.126-0.808) µg/m(3)).In Urumqi, source apportionment results for PM10 were soil sand dust and coal-combusted dust(49.75%), industry dust, vehicle emissions and secondary particles dust (30.65%). The main characteristic pollution element was Cd (0.463(0.033-1.351) ng/m(3)). As for PM2.5, the sources were soil sand dust and coal-combusted dust (43.26%), secondary particles dust (22.29%), industry dust and vehicle emissions (20.50%). The main characteristic pollution element was As (14.599 (1.696-36.741) µg/m(3)).In Qingdao, source apportionment results for PM10 were construction dust (30.91%), vehicle emissions and industry dust (29.65%) and secondary particles dust (28.99%). The main characteristic pollution element was Pb (64.071 (5.846-346.831) µg/m(3)). As for PM2.5, the sources were secondary particles dust, industry dust and vehicle emissions (49.82%) and construction dust (33.71%). The main characteristic pollution element was Pb(57.340 (5.004-241.559) µg/m(3)).Enrichment factors of Zn, Pb, As and Cd in PM2.5 were higher than those in PM10 both in Beijing and Urumqi. The major sources of the atmospheric particles PM10 and PM2.5 in Beijing were cement dust from construction sites and sand dust from soil; while the major sources of those in Urumqi were pollution by smoke and sand dust from burning coal. The major sources of the atmospheric particles PM10 in Qingdao were cement dust from construction sites; however, the major sources of PM2.5 there were secondary particles dust, industry dust and vehicle emissions. According to our study, the heavy metal elements were likely to gather in PM2.5.

Characterization of Dust Properties during ACE-Asia and PRIDE: A Column Satellite-Surface Perspective

NASA Technical Reports Server (NTRS)

Lau, William K. M. (Technical Monitor); Tsay, Si-Chee; Hsu, N. Christina; Herman, Jay R.; Ji, Q. Jack

2002-01-01

Many recent field experiments are designed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentration over particular pathways around the globe. For example, the ACE-Asia (Aerosol Characterization Experiment-Asia) was conducted from March-May 2001 in the vicinity of the Taklimakan and Gobi deserts, East Coast of China, Yellow Sea, Korea, and Japan, along the pathway of Kosa (severe events that blanket East Asia with yellow desert dust, peaked in the Spring season). The PRIDE (Puerto RIco Dust Experiment, July 2000) was designed to measure the properties of Saharan dust transported across the Atlantic Ocean to the Caribbean. Dust particles typically originate in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of dust aerosols is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the ocean. During ACE-Asia and PRIDE we had measured aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over homogeneous areas from ground-based remote sensing. The inclusion of flux measurements permits the determination of aerosol radiative flux in addition to measurements of loading and optical depth. At the time of the Terra/MODIS, SeaWiFS, TOMS and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. We will present the results and discuss their implications in regional climatic effects.

Importance of mineral dust and anthropogenic pollutants mixing during a long-lasting high PM event over East Asia.

PubMed

Wang, Zhe; Pan, Xiaole; Uno, Itsushi; Chen, Xueshun; Yamamoto, Shigekazu; Zheng, Haitao; Li, Jie; Wang, Zifa

2018-03-01

A long-lasting high particulate matter (PM) concentration episode persisted over East Asia from May 24 to June 3, 2014. The Nested Air Quality Prediction Model System (NAQPMS) was used to investigate the mixing of dust and anthropogenic pollutants during this episode. Comparison of observations revealed that the NAQPMS successfully reproduced the time series PM 2.5 and PM 10 concentrations, as well as the nitrate and sulfate concentrations in fine (aerodynamic diameter ≤ 2.5 μm) and coarse mode (2.5 μm < aerodynamic diameter ≤ 10 μm). This episode originated from two dust events that occurred in the inland desert areas of Mongolia and China, and then the long-range transported dust and anthropogenic pollutants were trapped over the downwind region of East Asia for more than one week due to the blocked north Pacific subtropical high-pressure system over the east of Japan. The model results showed that mineral dust accounted for 53-83% of PM 10 , and 39-67% of PM 2.5 over five cities in East Asia during this episode. Sensitivity analysis indicated that the Qingdao and Seoul regions experienced dust and pollution twice, by direct transport from the dust source region and from dust detoured over the Shanghai area. The results of the NAQPMS model confirmed the importance of dust heterogeneous reactions (HRs) over East Asia. Simulated dust NO 3 - concentrations accounted for 75% and 84% of total NO 3 - in fine and coarse mode, respectively, in Fukuoka, Japan. The horizontal distribution of model results revealed that the ratio of dust NO 3 - /dust concentration increased from about 1% over the Chinese land mass to a maximum of 8% and 6% respectively in fine and coarse mode over the ocean to the southeast of Japan, indicating that dust NO 3 - was mainly formed over the Yellow Sea and the East China Sea before reaching Japan. Copyright © 2017 Elsevier Ltd. All rights reserved.

Numerical simulation of "an American haboob"

NASA Astrophysics Data System (ADS)

Vukovic, A.; Vujadinovic, M.; Pejanovic, G.; Andric, J.; Kumjian, M. R.; Djurdjevic, V.; Dacic, M.; Prasad, A. K.; El-Askary, H. M.; Paris, B. C.; Petkovic, S.; Nickovic, S.; Sprigg, W. A.

2014-04-01

A dust storm of fearful proportions hit Phoenix in the early evening hours of 5 July 2011. This storm, an American haboob, was predicted hours in advance because numerical, land-atmosphere modeling, computing power and remote sensing of dust events have improved greatly over the past decade. High-resolution numerical models are required for accurate simulation of the small scales of the haboob process, with high velocity surface winds produced by strong convection and severe downbursts. Dust productive areas in this region consist mainly of agricultural fields, with soil surfaces disturbed by plowing and tracks of land in the high Sonoran Desert laid barren by ongoing draught. Model simulation of the 5 July 2011 dust storm uses the coupled atmospheric-dust model NMME-DREAM (Non-hydrostatic Mesoscale Model on E grid, Janjic et al., 2001; Dust REgional Atmospheric Model, Nickovic et al., 2001; Pérez et al., 2006) with 4 km horizontal resolution. A mask of the potentially dust productive regions is obtained from the land cover and the normalized difference vegetation index (NDVI) data from the Moderate Resolution Imaging Spectroradiometer (MODIS). The scope of this paper is validation of the dust model performance, and not use of the model as a tool to investigate mechanisms related to the storm. Results demonstrate the potential technical capacity and availability of the relevant data to build an operational system for dust storm forecasting as a part of a warning system. Model results are compared with radar and other satellite-based images and surface meteorological and PM10 observations. The atmospheric model successfully hindcasted the position of the front in space and time, with about 1 h late arrival in Phoenix. The dust model predicted the rapid uptake of dust and high values of dust concentration in the ensuing storm. South of Phoenix, over the closest source regions (~25 km), the model PM10 surface dust concentration reached ~2500 μg m-3, but underestimated the values measured by the PM10 stations within the city. Model results are also validated by the MODIS aerosol optical depth (AOD), employing deep blue (DB) algorithms for aerosol loadings. Model validation included Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO), equipped with the lidar instrument, to disclose the vertical structure of dust aerosols as well as aerosol subtypes. Promising results encourage further research and application of high-resolution modeling and satellite-based remote sensing to warn of approaching severe dust events and reduce risks for safety and health.

Capability of the CALIPSO lidar observations to detect the dust source regions

NASA Astrophysics Data System (ADS)

Kaskaoutis, D. G.; Kharol, Shailesh Kumar; Kambezidis, H. D.; Nastos, P. T.; Rani Sharma, Anu; Kvs, Badarinath

Two dust events with high aerosol optical depth (AOD) values have been observed over Athens on 4 and 6-7 February 2009. These dust events were well captured by the satellite obser-vations and are investigated in the present study by means of the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) observations, ceilometer vertical profiles and DREAM model predictions. The CALIPSO provides new insight to study the role of clouds and atmospheric aerosols in regulating Earth's weather, climate, and air quality. CALIPSO has a 98o-inclination orbit and flies at an altitude of 705 km providing daily global maps of the ver-tical distribution of aerosols and clouds. The CALIPSO satellite carries a polarization-sensitive lidar, the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), which provides profiles of backscatter coefficient at 532 and 1064 nm. The ceilometer used in the present study is a Vaisala CL31 model. It is equipped with an InGaAs MOCVD pulsed laser, emitting at 930 nm and having an energy per pulse of 1.2 J. The emission frequency is 10 kHz while the pulse duration is 100 ns. The vertical profiles of the aerosol backscatter coefficient were obtained from 5 m up to 7.5 km at 930 nm. The CL31 is installed at the Actinometric station of the National Observatory of Athens. The CALIPSO-derived total attenuated backscatter at 532 and 1064 nm is used to identify the position of dust along the overpass trajectory. A typical example of the vertical distribution of the dust plume over the study region during nighttime on 5 Febru-ary 2009 is provided. Limiting the analysis over Libya, eastern Mediterranean and Greece (24o -37o N, 15o-19o E), the dust aerosol layer exhibits a high total attenuated backscatter at 532 nm, reaching to 0.05-0.06 km-1sr-1. CALIPSO observations clearly show that the dust plume was generated over the Sahara desert at about 24oN, 15oE near the borders of Libya, Chad and Niger. After its exposure it was uplifted to about 3-km in depth and moved northwards. As the dust layer moved towards Greece its intensity seems to decrease while its vertical extent was limited to lower altitudes within the first 2 km. The ceilometer also detected an elevated aerosol layer due to dust transport within the first 3 km, while the vertical profiles of dust predicted by DREAM were in close agreement with those of the ceilometer. The main goal of this study is the investigation via satellite vertical-profiling instrumentation not only the vertical extent and the transport of dust, but also its source region. Keywords: Dust, CALIPSO, DREAM model and AOD

Greenland records of aerosol source and atmospheric lifetime changes from the Eemian to the Holocene.

PubMed

Schüpbach, S; Fischer, H; Bigler, M; Erhardt, T; Gfeller, G; Leuenberger, D; Mini, O; Mulvaney, R; Abram, N J; Fleet, L; Frey, M M; Thomas, E; Svensson, A; Dahl-Jensen, D; Kettner, E; Kjaer, H; Seierstad, I; Steffensen, J P; Rasmussen, S O; Vallelonga, P; Winstrup, M; Wegner, A; Twarloh, B; Wolff, K; Schmidt, K; Goto-Azuma, K; Kuramoto, T; Hirabayashi, M; Uetake, J; Zheng, J; Bourgeois, J; Fisher, D; Zhiheng, D; Xiao, C; Legrand, M; Spolaor, A; Gabrieli, J; Barbante, C; Kang, J-H; Hur, S D; Hong, S B; Hwang, H J; Hong, S; Hansson, M; Iizuka, Y; Oyabu, I; Muscheler, R; Adolphi, F; Maselli, O; McConnell, J; Wolff, E W

2018-04-16

The Northern Hemisphere experienced dramatic changes during the last glacial, featuring vast ice sheets and abrupt climate events, while high northern latitudes during the last interglacial (Eemian) were warmer than today. Here we use high-resolution aerosol records from the Greenland NEEM ice core to reconstruct the environmental alterations in aerosol source regions accompanying these changes. Separating source and transport effects, we find strongly reduced terrestrial biogenic emissions during glacial times reflecting net loss of vegetated area in North America. Rapid climate changes during the glacial have little effect on terrestrial biogenic aerosol emissions. A strong increase in terrestrial dust emissions during the coldest intervals indicates higher aridity and dust storm activity in East Asian deserts. Glacial sea salt aerosol emissions in the North Atlantic region increase only moderately (50%), likely due to sea ice expansion. Lower aerosol concentrations in Eemian ice compared to the Holocene are mainly due to shortened atmospheric residence time, while emissions changed little.

Rock-magnetic proxies of wind intensity and dust since 51,200 cal BP from lacustrine sediments of Laguna Potrok Aike, southeastern Patagonia

NASA Astrophysics Data System (ADS)

Lisé-Pronovost, Agathe; St-Onge, Guillaume; Gogorza, Claudia; Haberzettl, Torsten; Jouve, Guillaume; Francus, Pierre; Ohlendorf, Christian; Gebhardt, Catalina; Zolitschka, Bernd

2015-02-01

The sedimentary archive from Laguna Potrok Aike is the only continuous record reaching back to the last Glacial period in continental southeastern Patagonia. Located in the path of the Southern Hemisphere westerly winds and in the source region of dust deposited in Antarctica during Glacial periods, southern Patagonia is a vantage point to reconstruct past changes in aeolian activity. Here we use high-resolution rock-magnetic and physical grain size data from site 2 of the International Continental scientific Drilling Program (ICDP) Potrok Aike maar lake Sediment Archive Drilling prOject (PASADO) in order to develop magnetic proxies of dust and wind intensity at 52°S since 51,200 cal BP. Rock-magnetic analysis indicates the magnetic mineral assemblage is dominated by detrital magnetite. Based on the estimated flux of magnetite to the lake and comparison with distal dust records from the Southern Ocean and Antarctica, kLF is interpreted as a dust indicator in the dust source of southern Patagonia at the millennial time scale, when ferrimagnetic grain size and coercivity influence are minimal. Comparison to physical grain-size data indicates that the median destructive field of isothermal remanent magnetization (MDFIRM) mostly reflects medium to coarse magnetite bearing silts typically transported by winds for short-term suspension. Comparison with wind-intensity proxies from the Southern Hemisphere during the last Glacial period and with regional records from Patagonia since the last deglaciation including marine, lacustrine and peat bog sediments as well as speleothems reveals similar variability with MDFIRM up to the centennial time scale. MDFIRM is interpreted as a wind-intensity proxy independent of moisture changes for southeastern Patagonia, with stronger winds capable of transporting coarser magnetite bearing silts to the lake.

Characterisation of bio-aerosols during dust storm period in N-NW India

NASA Astrophysics Data System (ADS)

Yadav, Sudesh; Chauhan, M. S.; Sharma, Anupam

Bio-investigations for pollen and spores were performed on dry free-fall dust and PM 10 aerosol samples, collected from three different locations separated by a distance of 600 km, situated in dust storm hit region of N-NW India. Presence of pollen of trees namely Prosopis ( Prosopis juliflora and Prosopis cinearia), Acacia, Syzygium, Pinus, Cedrus, Holoptelea and shrubs namely Ziziphus, Ricinus, Ephedra and members of Fabaceae, Oleaceae families was recorded but with varying proportions in the samples of different locations. Poaceae, Chenopodiaceae/Amaranthaceae, Caryophyllaceae, Brassicaceae and Cyperaceae (sedges) were some of the herb pollen identified in the samples. Among the fungal spores Nigrospora was seen in almost all samples. Nigrospora is a well known allergen and causes health problems. The concentration of trees and shrubs increases in the windward direction just as the climate changes from hot arid to semiarid. The higher frequency of grasses (Poaceae) or herbs could either be a result of the presence of these herbs in the sampling area and hence the higher production of pollen/spores or due to the resuspension from the exposed surface by the high-intensity winds. But we cannot ascertain the exact process at this stage. The overall similarity in the pollen and spore assemblage in our dust samples indicates a common connection or source(s) to the dust in this region. Presence of the pollen of the species of Himalayan origin in our entire samples strongly point towards a Himalayan connection, could be direct or indirect, to the bioaerosols and hence dust in N-NW India. In order to understand the transport path and processes involved therein, present study needs further extension with more number of samples and with reference to meteorological parameters.

Heavy metal speciation in various grain sizes of industrially contaminated street dust using multivariate statistical analysis.

PubMed

Yıldırım, Gülşen; Tokalıoğlu, Şerife

2016-02-01

A total of 36 street dust samples were collected from the streets of the Organised Industrial District in Kayseri, Turkey. This region includes a total of 818 work places in various industrial areas. The modified BCR (the European Community Bureau of Reference) sequential extraction procedure was applied to evaluate the mobility and bioavailability of trace elements (Cd, Co, Cr, Cu, Fe, Mn, Ni, Pb and Zn) in street dusts of the study area. The BCR was classified into three steps: water/acid soluble fraction, reducible and oxidisable fraction. The remaining residue was dissolved by using aqua regia. The concentrations of the metals in street dust samples were determined by flame atomic absorption spectrometry. Also the effect of the different grain sizes (<38µm, 38-53µm and 53-74µm) of the 36 street dust samples on the mobility of the metals was investigated using the modified BCR procedure. The mobility sequence based on the sum of the first three phases (for <74µm grain size) was: Cd (71.3)>Cu (48.9)>Pb (42.8)=Cr (42.1)>Ni (41.4)>Zn (40.9)>Co (36.6)=Mn (36.3)>Fe (3.1). No significant difference was observed among metal partitioning for the three particle sizes. Correlation, principal component and cluster analysis were applied to identify probable natural and anthropogenic sources in the region. The principal component analysis results showed that this industrial district was influenced by traffic, industrial activities, air-borne emissions and natural sources. The accuracy of the results was checked by analysis of both the BCR-701 certified reference material and by recovery studies in street dust samples. Copyright © 2015 Elsevier Inc. All rights reserved.

Attic Dust Analysis Approach for Evaluation of Heavy Metal Deposition on the El Paso Del Norte Region

NASA Astrophysics Data System (ADS)

Shekhter, E. G.; van Pelt, S.; Pannell, K.; Gill, T. E.; Barnes, M. A.

2010-12-01

The El Paso del Norte region in the United States is a region of complex topography that is the home to more than 2 million people who share the same air. A large non-ferrous smelter (primary lead-copper smelter),owned by the American Smelting and Refining Company (ASARCO), was functioning in the Rio Grande River valley on the west side of the Franklin Mountains that divide the city of El Paso and across the river from Juarez, Mexico’s largest city on the United States border. During the more than 100 years of operation, beginning in 1887, the ASARCO smelter emissions considerably deteriorated the already complex environmental condition on the US-Mexican border. In order to identify the sources and patterns of heavy metal dispersion, we used an attic dust analyses approach which has not been previously been applied in this area. Undisturbed attic dust can provide an integrated history of atmospheric loading of particulates emanating from geological, biological and anthropogenic sources and can help to reconstruct the air pollution history on a local scale. We sampled attic dust and dust from undisturbed surfaces in 15 buildings of varying ages from three neighborhoods in the cities of El Paso and Juarez. The dust samples and samples of unpolluted buried soil horizons in the area were extracted with aqua regia and analyzed by ICP-AES and ICP-MS. Enrichment ratios (ER) were calculated by dividing the concentration of a trace metal in the attic dust by the mean concentration of the same element in the buried soil horizons. Mean ER for Pb were 263.3, 95.4, and 70.2 for dust collected in a neighborhood near the smelter, downtown Juarez, and an El Paso neighborhood on the other side of the Franklin Mountains from the smelter. Greater ER for As, Cd, Zn, Sb, and Cu followed the same trends, by neighborhood, noted for Pb. In addition, dust collected from attics surfaces (pipes, ducts, storage containers) post-dating smelter disclosure had lower ER for the trace metals than samples collected on adjacent surfaces that were present during the period of smelter operation. Based on the evidence provided by dust chemistry, we conclude that heavy metal contamination was predominantly from smelter stack emissions, was preferentially deposited on the near field, and generally followed the lower path provided by Rio Grande valley rather than mixing to heights that could result in movement over the Franklin Mountains and deposition on the east side of El Paso.

Development of a dust deposition forecast model for a mine tailings impoundment

NASA Astrophysics Data System (ADS)

Stovern, Michael

Wind erosion, transport and deposition of particulate matter can have significant impacts on the environment. It is observed that about 40% of the global land area and 30% of the earth's population lives in semiarid environments which are especially susceptible to wind erosion and airborne transport of contaminants. With the increased desertification caused by land use changes, anthropogenic activities and projected climate change impacts windblown dust will likely become more significant. An important anthropogenic source of windblown dust in this region is associated with mining operations including tailings impoundments. Tailings are especially susceptible to erosion due to their fine grain composition, lack of vegetative coverage and high height compared to the surrounding topography. This study is focused on emissions, dispersion and deposition of windblown dust from the Iron King mine tailings in Dewey-Humboldt, Arizona, a Superfund site. The tailings impoundment is heavily contaminated with lead and arsenic and is located directly adjacent to the town of Dewey-Humboldt. The study includes in situ field measurements, computational fluid dynamic modeling and the development of a windblown dust deposition forecasting model that predicts deposition patterns of dust originating from the tailings impoundment. Two instrumented eddy flux towers were setup on the tailings impoundment to monitor the aeolian and meteorological conditions. The in situ observations were used in conjunction with a computational fluid dynamic (CFD) model to simulate the transport of windblown dust from the mine tailings to the surrounding region. The CFD model simulations include gaseous plume dispersion to simulate the transport of the fine aerosols, while individual particle transport was used to track the trajectories of larger particles and to monitor their deposition locations. The CFD simulations were used to estimate deposition of tailings dust and identify topographic mechanisms that influence deposition. Simulation results indicated that particles preferentially deposit in regions of topographic upslope. In addition, turbulent wind fields enhanced deposition in the wake region downwind of the tailings. This study also describes a deposition forecasting model (DFM) that can be used to forecast the transport and deposition of windblown dust originating from a mine tailings impoundment. The DFM uses in situ observations from the tailings and theoretical simulations of aerosol transport to parameterize the model. The model was verified through the use of inverted-disc deposition samplers. The deposition forecasting model was initialized using data from an operational Weather Research and Forecasting (WRF) model and the forecast deposition patterns were compared to the inverted-disc samples through gravimetric, chemical composition and lead isotopic analysis. The DFM was verified over several month-long observing periods by comparing transects of arsenic and lead tracers measured by the samplers to the DFM PM27 forecast. Results from the sampling periods indicated that the DFM was able to accurately capture the regional deposition patterns of the tailings dust up to 1 km. Lead isotopes were used for source apportionment and showed spatial patterns consistent with the DFM and the observed weather conditions. By providing reasonably accurate estimates of contaminant deposition rates, the DFM can improve the assessment of human health impacts caused by windblown dust from the Iron King tailings impoundment.

The near-infrared broad emission line region of active galactic nuclei - II. The 1-μm continuum

NASA Astrophysics Data System (ADS)

Landt, Hermine; Elvis, Martin; Ward, Martin J.; Bentz, Misty C.; Korista, Kirk T.; Karovska, Margarita

2011-06-01

We use quasi-simultaneous near-infrared (near-IR) and optical spectroscopy from four observing runs to study the continuum around 1 μm in 23 well-known broad emission line active galactic nuclei (AGN). We show that, after correcting the optical spectra for host galaxy light, the AGN continuum around this wavelength can be approximated by the sum of mainly two emission components, a hot dust blackbody and an accretion disc. The accretion disc spectrum appears to dominate the flux at ˜ 1 μm, which allows us to derive a relation for estimating AGN black hole masses based on the near-IR virial product. This result also means that a near-IR reverberation programme can determine the AGN state independent of simultaneous optical spectroscopy. On average we derive hot dust blackbody temperatures of ˜1400 K, a value close to the sublimation temperature of silicate dust grains, and relatively low hot dust covering factors of ˜7 per cent. Our preliminary variability studies indicate that in most sources, the hot dust emission responds to changes in the accretion disc flux with the expected time lag; however, a few sources show a behaviour that can be attributed to dust destruction.

Far-Infrared sources and diffuse emission in M31

NASA Technical Reports Server (NTRS)

Xu, Cong; Helou, George

1994-01-01

A study on the far-infrared (FIR) emission of M31 has been carried out with the High Resolution (HiRes) maps (approx. 1 min) derived from IRAS data. Sixty-eight FIR sources are detected in M31, which in general coincide with optical HII regions, and contribute 15, 23, 29, and 23 percent to the fluxes in 12, 25, 60, and 100 micron bands, respectively. The remaining diffuse emission, which dominates the FIR emission of M31, is studied using a dust heating model which utilizes the UV and optical photometry maps and the HI maps available in the literature. It is found that the global dust-to-gas ratio in M31 disk is 6.5 10(exp -3), very close to the dust-to-gas ratio in the solar neighborhood. There is a significant galactocentric gradient of the dust-to-HI-gas ratio, with an e-folding scale length of 9 kpc. The diffuse dust correlates tightly with the HI gas. The model indicates that the non-ionizing UV (913-4000A) radiation from massive and intermediate massive stars contributes only about 30 percent of the heating of the diffuse dust, while the optical-NIR (4000-9000A) radiation from the old stellar population is responsible for the most of the heating.

Climate Effects and Efficacy of Dust and Soot in Snow

NASA Astrophysics Data System (ADS)

Zender, C. S.; Flanner, M. G.; Randerson, J. T.; Mahowald, N. M.; Rasch, P. J.; Yoshioka, M.; Painter, T.

2006-12-01

Dust and industrial and biomass burning emissions from low and mid-latitudes dominate the absorbing impurities trapped in snow at mid- and high-latitudes. We study the effects of dust and smoke on global and regional climate using a general circulation model driven by observed and predicted aerosol emissions determined from satellite and in situ observations. The model has sophisticated treatments of aerosol and snowpack radiative and thermodynamic processes that compare well with observations of snow albedo evolution and impurity concentration. This presentation focuses on the individual and combined contributions of present day dust and soot to snow-albedo forcing and on the global temperature and snowpack responses. Results are emphasized near India and East Asia, where the anthropogenic aerosol forcing of surface albedo and hydrology is greatest. We find that dust and black carbon (BC) aerosols have climate change efficacies (surface temperature change per unit forcing) about 3--4 times greater than CO2, making them the most efficacious forcing agents known. We estimate present day dust and soot snowpack-forcing of ~ 0.050 W m-2 warms global climate by ~ 0.16 °K. Anthropogenic soot from fossil fuel sources causes more than 50% of this warming, and biomass burning can account for up to 30% in strong tropical or boreal burn years. The greatest forcings occur in the Tarim/Mongol region (due to dust), northeastern China (due to soot), and the Tibetan Plateau (both). Dirty springtime snow in these regions can darken albedo by more than 0.1 and increase surface absorption by more than 20 W m-2. These results have implications for the strength of the Asian Monsoon, which is negatively correlated with antecedent snow cover in non-ENSO years. Dust and soot have such strong efficacies because they increase spring melt rates thus reduce summer snow cover. In some regions and seasons, dirty snow reduces snowpack depth and cover by 50%, triggering strong snow and sea-ice albedo feedbacks.

77 FR 11798 - Approval and Promulgation of Air Quality Implementation Plans; Rhode Island; Regional Haze

Federal Register 2010, 2011, 2012, 2013, 2014

2012-02-28

...; and Lye Brook Wilderness Area in Vermont. Through source apportionment modeling, MANE-VU assisted... sources and activities which are located across a broad geographic area and emit fine particles and their...., sulfates, nitrates, organic carbon, elemental carbon, and soil dust), which also impair visibility by...

Characterization of east Asian dust outbreaks in the spring of 2001 using ground-based and satellite data

NASA Astrophysics Data System (ADS)

Darmenova, Kremena; Sokolik, Irina N.; Darmenov, Anton

2005-01-01

This study presents a detailed examination of east Asian dust events during March-April of 2001, by combining satellite multisensor observation (Total Ozone Mapping Spectrometer (TOMS), Moderate-Resolution Imaging Spectroradiometer (MODIS), and Sea-Viewing Wide Field-of-View Sensor (SeaWiFS)) meteorological data from weather stations in China and Mongolia and the Pennsylania State University/National Center for Atmospheric Research Mesoscale Modeling System (MM5) driven by the National Centers for Environmental Prediction Reanalysis data. The main goal is to determine the extent to which the routine surface meteorological observations (including visibility) and satellite data can be used to characterize the spatiotemporal distribution of dust plumes at a range of scales. We also examine the potential of meteorological time series for constraining the dust emission schemes used in aerosol transport models. Thirty-five dust events were identified in the source region during March and April of 2001 and characterized on a case-by-case basis. The midrange transport routes were reconstructed on the basis of visibility observations and observed and MM5-predicted winds with further validation against satellite data. We demonstrate that the combination of visibility data, TOMS aerosol index, MODIS aerosol optical depth over the land, and a qualitative analysis of MODIS and SeaWiFS imagery enables us to constrain the regions of origin of dust outbreaks and midrange transport, though various limitations of individual data sets were revealed in detecting dust over the land. Only two long-range transport episodes were found. The transport routes and coverage of these dust episodes were reconstructed by using MODIS aerosol optical depth and TOMS aerosol index. Our analysis reveals that over the oceans the presence of persistent clouds poses a main problem in identifying the regions affected by dust transport, so only partial reconstruction of dust transport routes reaching the west coast of the United States was possible.

Conditions and Dynamics Within a Regional Mars Dust Storm

NASA Astrophysics Data System (ADS)

Rafkin, S. C.; Pla-García, J.; Leung, C. W. S.

2017-12-01

There have never been in situ observations at or near the active lifting center of a regional dust storm on Mars. In the absence of in situ data, it is common to employ numerical models to provide guidance on the physical processes and conditions operating in an unobserved location or weather system. Consequently, the Mars Regional Atmospheric Modeling System (MRAMS) is employed to study the structure and dynamics of a simulated large regional storm using a fully interactive dust cycle. The simulations provide the first ever glimpse of the conditions that might occur inside one of these storms. The simulated storm shows extremely complex structure, highly heterogeneous lifting centers, and a variety of deep dust transport circulations. The active lifting centers show broader organization into a mesoscale system in much the same way that thunderstorms on Earth can organize into mesoscale convective structures. In many of the active dust plumes, the mixing ratio of dust peaks near the surface and drops off with height. The surface mixing ratio maximum is partly due to the surface being the source of dust, with entrainment of less dusty air as the plume rises. However, it is also because the mixing ratio can be dominated by a few large dust aerosol, since the mass is proportional to the cubed of the radius. Once lifted, the largest dust tends to sediment out while the smaller dust continues to be advected upward by the plume. This size-sorting process tends to drive the mixing ratio profile to a maximum near the surface. In dusty plumes near the surface, the air temperature is as much as 20K colder than nearby areas. This is due to solar absorption higher in the dust column limiting direct heating deeper into the atmosphere. Overall, within the plume, there is an inversion, and although the top of the plume is warmer than below, it is near neutral buoyancy compared to the less dusty air on either side. Apparently, adiabatic cooling nearly offsets the expected positive heating perturbation at the top of the dusty plume. A very strong low level just forms in the vicinity of the storm, accompanied by system-wide negative pressure deficits and circulation patterns strongly suggestive of the wind-enhanced interaction of radiation and dust (WEIRD) feedback mechanism.

Saharan dust - A carrier of persistent organic pollutants, metals and microbes to the Caribbean?

USGS Publications Warehouse

Garrison, V.H.; Foreman, W.T.; Genualdi, S.; Griffin, Dale W.; Kellogg, C.A.; Majewski, M.S.; Mohammed, A.; Ramsubhag, A.; Shinn, E.A.; Simonich, S.L.; Smith, G.W.

2006-01-01

An international team of scientists from government agencies and universities in the United States, U.S. Virgin Islands (USVI), Trinidad & Tobago, the Republic of Cape Verde, and the Republic of Mali (West Africa) is working together to elucidate the role Saharan dust may play in the degradation of Caribbean ecosystems. The first step has been to identify and quantify the persistent organic pollutants (POPs), trace metals, and viable microorganisms in the atmosphere in dust source areas of West Africa, and in dust episodes at downwind sites in the eastern Atlantic (Cape Verde) and the Caribbean (USVI and Trinidad & Tobago). Preliminary findings show that air samples from Mali contain a greater number of pesticides, polychlorinated biphenyls (PCBs) and polycyclic aromatic hydrocarbons (PAHs) and in higher concentrations than the Caribbean sites. Overall, POP concentrations were similar in USVI and Trinidad samples. Trace metal concentrations were found to be similar to crustal composition with slight enrichment of lead in Mali. To date, hundreds of cultureable micro-organisms have been identified from Mali, Cape Verde, USVI, and Trinidad air samples. The sea fan pathogen, Aspergillus sydowii, has been identified in soil from Mali and in air samples from dust events in the Caribbean. We have shown that air samples from a dust-source region contain orders of magnitude more cultureable micro-organisms per volume than air samples from dust events in the Caribbean, which in turn contain 3-to 4-fold more cultureable microbes than during non-dust conditions.

An aerosol climatology for a rapidly growing arid region (southern Arizona): Major aerosol species and remotely sensed aerosol properties

NASA Astrophysics Data System (ADS)

Sorooshian, Armin; Wonaschütz, Anna; Jarjour, Elias G.; Hashimoto, Bryce I.; Schichtel, Bret A.; Betterton, Eric A.

2011-10-01

This study reports a comprehensive characterization of atmospheric aerosol particle properties in relation to meteorological and back trajectory data in the southern Arizona region, which includes two of the fastest growing metropolitan areas in the United States (Phoenix and Tucson). Multiple data sets (MODIS, AERONET, OMI/TOMS, MISR, GOCART, ground-based aerosol measurements) are used to examine monthly trends in aerosol composition, aerosol optical depth (AOD), and aerosol size. Fine soil, sulfate, and organics dominate PM2.5 mass in the region. Dust strongly influences the region between March and July owing to the dry and hot meteorological conditions and back trajectory patterns. Because monsoon precipitation begins typically in July, dust levels decrease, while AOD, sulfate, and organic aerosol reach their maximum levels because of summertime photochemistry and monsoon moisture. Evidence points to biogenic volatile organic compounds being a significant source of secondary organic aerosol in this region. Biomass burning also is shown to be a major contributor to the carbonaceous aerosol budget in the region, leading to enhanced organic and elemental carbon levels aloft at a sky-island site north of Tucson (Mt. Lemmon). Phoenix exhibits different monthly trends for aerosol components in comparison with the other sites owing to the strong influence of fossil carbon and anthropogenic dust. Trend analyses between 1988 and 2009 indicate that the strongest statistically significant trends are reductions in sulfate, elemental carbon, and organic carbon, and increases in fine soil during the spring (March-May) at select sites. These results can be explained by population growth, land-use changes, and improved source controls.

Aerosol Source Attributions and Source-Receptor Relationships Across the Northern Hemisphere

NASA Technical Reports Server (NTRS)

Bian, Huisheng; Chin, Mian; Kucsera, Tom; Pan, Xiaohua; Darmenov, Anton; Colarco, Peter; Torres, Omar; Shults, Michael

2014-01-01

Emissions and long-range transport of air pollution pose major concerns on air quality and climate change. To better assess the impact of intercontinental transport of air pollution on regional and global air quality, ecosystems, and near-term climate change, the UN Task Force on Hemispheric Transport of Air Pollution (HTAP) is organizing a phase II activity (HTAP2) that includes global and regional model experiments and data analysis, focusing on ozone and aerosols. This study presents the initial results of HTAP2 global aerosol modeling experiments. We will (a) evaluate the model results with surface and aircraft measurements, (b) examine the relative contributions of regional emission and extra-regional source on surface PM concentrations and column aerosol optical depth (AOD) over several NH pollution and dust source regions and the Arctic, and (c) quantify the source-receptor relationships in the pollution regions that reflect the sensitivity of regional aerosol amount to the regional and extra-regional emission reductions.

Enigmatic Extinction: An Investigation of the 2175Å Extinction Bump in M101

NASA Astrophysics Data System (ADS)

Danowski, Meredith E.; Cook, Timothy; Gordon, Karl D.; Chakrabarti, Supriya; Lawton, Brandon L.; Misselt, Karl A.

2014-06-01

Evidence from studies of starburst galaxies indicates that active formation of high mass stars modifies the UV dust extinction curve as seen by a lack of the characteristic 2175Å bump. For over 45 years, the source of the 2175Å extinction feature has yet to be positively identified. Small aromatic/PAH grains are suggested as a leading contender in dust grain models. The face-on spiral galaxy M101 is an ideal laboratory for the study of dust, with many well-studied HII regions and a steep metallicity and ionization gradient.The Interstellar Medium Absorption Gradient Experiment Rocket (IMAGER) probes the correlation between dust extinction, and the metallicity and radiation environment in M101 at ultraviolet wavelengths. IMAGER simultaneously images M101 in three 400Å-wide bandpasses, measuring the apparent strength of the 2175Å bump and the UV continuum.Combining data from IMAGER with high S/N far- and near- UV observations from the MAMA detectors on the Hubble STIS instrument, we examine the apparent strength of the 2175Å bump in HII regions of M101. With additional infrared data from Spitzer, the DIRTY radiative transfer model, and stellar evolution models, we probe the correlation between the 2175Å feature and the aromatic/PAH features across HII regions of varying metallicity and radiation field hardness. The results of this experiment will directly impact our understanding of the nature of dust and our ability to accurately account for the effects of dust on observations at all redshifts.

A multi-wavelength investigation of Seyfert 1.8 and 1.9 galaxies

NASA Astrophysics Data System (ADS)

Trippe, Margaret L.

We focus on determining the underlying physical cause of a Seyfert galaxy's appearance as type a 1.8 or 1.9. Are these "intermediate" Seyfert types typical Seyfert 1 nuclei reddened by central dusty tori or by nuclear dust lanes/spirals in the narrow-line region? Or, are they similar to NGC 2992, objects that have intrinsically weak continua and weak broad emission lines? Our study compares measurements of the reddenings of the narrow and broad-line regions with each other and with the X-ray column derived from XMM Newton 0.5--10 keV spectra to determine the presence and location of dust in the line of sight for a sample of 35 Seyfert 1.8s and 1.9s. From this, we find that Seyfert 1.9s are an almost equal mix of low-flux objects with unreddened broad line regions, and objects with broad line regions reddened by an internal dust source, either the torus or dust structures on the same size scale as the narrow line region. The 1.9s that recieved this designation due to a low continuum flux state showed variable type classifications. All three of the Seyfert 1.8s in our study are probably in low continuum states. Many objects have been misclassified as Seyfert 1.8/1.9s in the past, probably due to improper [N II]/Halpha deconvolution leading to a false detection of weak broad Halpha. INDEX WORDS: Active galaxies, Seyfert galaxies, Optical spectroscopy, X-ray spectroscopy, Astronomical dust

A 16-year record of eolian dust in Southern Nevada and California, USA: Controls on dust generation and accumulation

USGS Publications Warehouse

Reheis, M.C.

2006-01-01

An ongoing project monitors modern dust accumulation in the arid southwestern United States to (1) determine the rate and composition of dust inputs to soils and (2) relate dust accumulation to weather patterns to help predict the effects of climate change on dust production and accumulation. The 16-year records of 35 dust-trap sites in the eastern Mojave Desert and southern Great Basin reveal how generation and accumulation of dust, including the silt-clay, carbonate, and soluble-salt fractions, is affected by the amount and seasonal distribution of rainfall and the behavior of different source types (alluvium, dry playas, and wet playas). Accumulation rates (fluxes) of the silt-clay fraction of dust, including carbonates, range from about 2-20 g/m2/yr. Average rates are higher in the southern part of the study area (south of latitude 36.5??N) and annually fluctuate over a larger range than rates in the northern part of the area. Sites throughout the study area show peaks in dust flux in the 1984-1985 sampling period and again in 1997-1999; northern sites also show increased flux in 1987-1988 and southern sites in 1989-1991. These peaks of dust flux correspond with both La Nina (dry) conditions and with strong El Nino (wet) periods. The accumulation rates of different components of mineral dusts fluctuate differently. For example, soluble-salt flux increases in 1987-1988, coincident with a moderate El Nino event, and increases very strongly in 1997-1999, overlapping with a strong El Nino event. Both of these high-rainfall winters were preceded and accompanied by strong summer rains. In contrast, little or no change in soluble-salt flux occurred during other periods of high winter rainfall but little summer rain, e.g. 1992-1995. The differences between northern vs. southern sites and between sites with playa dust sources vs. alluvial dust sources indicate that regional differences in the response of precipitation and vegetation growth to ENSO influence and differences in the response of source types control dust production and accumulation. A major factor is the hydrologic condition of surface sediments. The silt-clay and soluble-salt fluxes increased during the El Nino events of 1987-1988 and 1997-1998 at sites close to "wet" playas with shallow depths to groundwater (<10 m), consistent with the concept that active evaporative concentration of salts disrupts surface crusts and increases the susceptibility of surface sediment to deflation. The silt-clay flux also increased during drought periods (1989-1991, 1995-1997) at sites downwind of alluvial sources and "dry" playas with deeper groundwater (<10 m). These increases are probably related to the die-off of drought-stressed vegetation on alluvial sediments, and in some cases to local runoff events that deliver fresh sediment to playa margins and distal portions of alluvial fans. ?? 2006 Elsevier Ltd. All rights reserved.

Dust Deposition and Migration of the ITCZ through the Last Glacial Cycle in the Central Equatorial Pacific (Line Islands).

NASA Astrophysics Data System (ADS)

Reimi Sipala, M. A.; Marcantonio, F.

2014-12-01

Atmospheric dust can be used to record climate change in addition to itself playing a role in several key climate processes, such as affecting Earth's albedo, fomenting rain coalescence, encouraging biological productivity, and enhancing carbon export though particle sinks. Using deep sea sediments, it is possible to quantify and locate the sources and sinks of atmospheric dust. A key area of research is the shift in the inter-tropical converge zone (ITCZ), a thermally influenced area that shifts according to the northern and southern hemisphere temperature gradient. This ongoing project focuses on the changes of the ITCZ over the Central Equatorial Pacific (CEP) over the past ~25000 years. The research focuses on two cores taken from the Line Islands Ridge at 0° 29' N (ML1208-18GC), and 4° 41' N (ML1208-31BB). The main aim is to quantify the magnitude and provenance of windblown dust deposited in the CEP, and to address questions regarding the nature of the variations of dust through ice-age climate transitions. Radiogenic isotopes (Sr, Nd, Pb) have been successfully used to distinguish between different potential dust sources in the aluminosilicates fractions of Pacific Sediments. Our preliminary Pb isotope ratios suggest that, for modern deposition, the northern core's (31BB) detrital sediment fraction is likely sourced from Asian Loess (average ratios are 206Pb/204Pb = 18.88, 207Pb/204Pb = 15.69, 208Pb/204Pb = 39.06). The equatorial core's (18GC) detrital fraction has a less radiogenic Pb signature, which is consistent with South American dust sourcing (206Pb/204Pb = 18.62, 207Pb/204Pb = 15.63, 208Pb/204Pb = 38.62). This is indicative of a strong modern ITCZ that acts as an effective barrier for inter-hemispheric dust transport. Prior to Holocene time, the changes in Pb isotope ratios in both cores appear to be in anti-phase; the northern core becomes less radiogenic up to the LGM, while the southern core becomes more radiogenic. This is potentially due to a weakening of the ITCZ during glacial times. Future work on Nd isotope will shed additional light on subtle differences in dust isotopic composition within the source regions of interest, including the different volcanic zones of South America.

Lyman alpha radiation in external galaxies

NASA Technical Reports Server (NTRS)

Neufeld, David A.; Mckee, Christopher F.

1990-01-01

The Ly alpha line of atomic hydrogen is often a luminous component of the radiation emitted by distant galaxies. Except for those galaxies which have a substantial central source of non-stellar ionizing radiation, most of the Ly alpha radiation emitted by galaxies is generated within regions of the interstellar medium which are photoionized by starlight. Conversely, much of the energy radiated by photoionized regions is carried by the Ly alpha line. Only hot, massive stars are capable of ionizing hydrogen in the interstellar medium which surrounds them, and because such stars are necessarily short-lived, Ly alpha emission traces regions of active star formation. Researchers argue that the strength of the Ly alpha emission observed from external galaxies may be used to estimate quantitatively the dust content of the emitting region, while the Ly alpha line profile is sensitive to the presence of shock waves. Interstellar dust particles and shock waves are intimately associated with the process of star formation in two senses. First, both dust particles and shock waves owe their existence to stellar activity; second, they may both serve as agents which facilitate the formation of stars, shocks by triggering gravitational instabilities in the interstellar gas that they compress, and dust by shielding star-forming molecular clouds from the ionizing and dissociative effects of external UV radiation. By using Ly alpha observations as a probe of the dust content in diffuse gas at high redshift, we might hope to learn about the earliest epochs of star formation.

Impact of long-range transport pollution on aerosol properties over West Africa: observations during the DACCIWA airborne campaign

NASA Astrophysics Data System (ADS)

Denjean, Cyrielle; Bourrianne, Thierry; Burnet, Frederic; Deroubaix, Adrien; Brito, Joel; Dupuy, Régis; Colomb, Aurélie; Schwarzenboeck, Alfons; Sellegri, Karine; Chazette, Patrick; Duplissy, Jonathan; Flamant, Cyrille

2017-04-01

Southern West Africa (SWA) is a region highly vulnerable to climate change. Emissions of anthropogenic pollution have increased substantially over the past decades in the region and are projected to keep increasing. The region is also strongly impacted by important natural pollution from distant locations. Biomass burning mainly from vegetation fires in Central Africa and mineral dust from the Saharan and Sahel-Sudan regions are advected by winds to the SWA region especially in summer. Both biomass burning and mineral dust aerosols scatter and absorb solar radiation and are able to significantly modify the regional radiative budget. Presently, the potential radiative impact of dust and biomass burning particles on SWA is unclear due to inadequate data information on the aerosols properties and vertical distribution. In the framework of the Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa (DACCIWA) project, an unprecedented field campaign took place in summer 2016 in West Africa. The ATR-42 research aircraft operated by SAFIRE performed twenty flights to sample the local air pollution from maritime traffic and coastal megacities, as well as regional pollution from biomass burning and desert dust. The aircraft was equipped with state of the art in situ instrumentation to measure the aerosol optical properties (CAPS, nephelometer, PSAP), the aerosol size distribution (SMPS, GRIMM, USHAS, PCASP, FSSP) and the aerosol chemical composition (SP2, AMS). A mini backscattered lidar system provided additional measurements of the aerosol vertical structure and the aerosol optical properties such as the particulate depolarization ratio. The CHIMERE chemistry and transport model has been used to characterize the source area and the long-range transport of dust and biomass burning plumes. Here, we investigate the aerosol microphysical, chemical and optical properties of biomass burning and dust aerosols transported in SWA. In particular the following questions will be addressed: (i) what are the differences in the aerosol optical properties and vertical distribution in SWA during intense biomass burning and dust events ? (ii) what is the range of mass extinction efficiencies and single scattering albedo for these events and what explains their variability ? (iii) what is the range in aerosol size distribution in biomass burning and dust layers and how does this vary with plume age ?

African dust outbreaks over the Mediterranean Basin during 2001-2011: concentrations, phenomenology and trends

NASA Astrophysics Data System (ADS)

Pey, Jorge; Querol, Xavier; Alastuey, Andres; Forastiere, Franceso; Stafoggia, Massimo

2013-04-01

Concentrations, phenomenology and trends of African dust outbreaks over the whole Mediterranean Basin werestudied on an 11-year period (2001-2011). This work has been performed in the context of the MED-PARTICLES (LIFE programme, EU) project, devoted to quantify short-term health effects of particulate matter over the Mediterranean region by distinguishing different particle sizes, chemical components and sources, with emphasis in the effects of African dust. In order to evaluate conduct this investigation, PM10 data from 19 regional and suburban background sites West to East in the Mediterranean area were compiled. After identifying the daily occurrence of African dust outbreaks, a methodology for estimating natural dust contributions on daily PM10 concentrations was applied. Our findings point out that African dust outbreaks are sensibly more frequent in southern sitesacross the Mediterranean, from 30 to 37 % of the annual days, whereas they occur less than 20% of the annual days in northern sites. The central Mediterranean emerges as a transitional area, with slightly higher frequency of dust episodes in its lower extreme when compared to similar latitudinal positions in western and eastern sides of the Basin. A decreasing south to north gradient of African dust contribution to PM10, driven by the latitudinal position of the monitoring sites at least 25°E westwards across the Basin,is patent across the Mediterranean. From 25°E eastwards, higher annual dust contributions are encountered due to the elevated annual occurrence of severe episodesof dust but also because of inputs from Middle Eastern deserts. Concerning seasonality patterns and intensity characteristics, a clear summer prevalence is observed in the western part, with low occurrence of severe episodes (daily dust averages over 100 µg m-3 in PM10); no seasonal trend is detected in the central region, with moderate-intensity episodes; and significantly higher contributions are common in autumn-spring in the eastern side, with occurrence of various severe episodes throughout the year. Overall, African dust emerges as the largest PM10 source in regional background southern sites of the Mediterranean (35-50% of PM10), with seasonal peak contributions to PM10 up to 80% of the total mass in the eastern side. The multi-year study of African dust episodes and their contributions to PM10 concentrations displaysa consistent decreasing trend in the period 2006/2007 to 2011 in 4 of the 17 studied regions, all of them located in the NW of the Mediterranean. Such decrease is almost parallel to that of NAO (North Atlantic Oscillation) index for the summer period, being progressively more negative since 2006. As a consequence, a sharp change in the atmospheric circulation over the last 5 years (a similar negative NAO period occurred in the 1950 decade) have affected the number of African dust episodes and consequently the annual dust inputs to PM10observed in the NW part of the Mediterranean. By investigating mean temperatures and geopotential height maps at 850hPa it is evident a displacement of warm air masses accomplishing African dust towards the central Mediterranean in the 2007-2008 period, and towards the NW African coast and the Canary Islands in the 2009-2011 period. Acknowledgements This study has been founded by the LIFE programme of the European Commission under the Grant Agreement LIFE10 ENV/IT/327. Partial founding was received from the Autonomous Government of Catalonia and the Spanish Ministry of Agriculture, Food and Environment. PM10 data were obtained from EMEP, Airbase and ACTRIS databases. Most of the interpretations were performed thanks to the support of HYSPLIT model, SKIRON, BSC-DREAM and NRL-NAAPS aerosol maps, NCEP/NCAR meteorological database, and image products from MODIS and SeaWiFs NASA satellites.

Links between Patagonian Ice Sheet fluctuations and Antarctic dust variability during the last glacial period (MIS 4-2)

NASA Astrophysics Data System (ADS)

Kaiser, Jérôme; Lamy, Frank

2010-06-01

Antarctic and Greenland ice-core records reveal large fluctuations of dust input on both orbital and millennial time-scales with potential global climate implications. At least during glacial periods, the Antarctic dust fluctuations appear to be largely controlled by environmental changes in southern South America. We compare dust flux records from two Antarctic ice-cores to variations in the composition of the terrigenous supply at ODP Site 1233 located off southern Chile and known to record fluctuations in the extent of the northern part of the Patagonian ice-sheet (NPIS) during the last glacial period (Marine Isotope Stage, MIS, 4 to 2). Within age uncertainties, millennial-scale glacial advances (retreats) of the NPIS correlate to Antarctic dust maxima (minima). In turn, NPIS fluctuations were closely related to offshore sea surface temperature (SST) changes. This pattern suggests a causal link involving changes in temperature, in rock flour availability, in latitudinal extensions of the westerly winds and in foehn winds in the southern Pampas and Patagonia. We further suggest that the long-term trend of dust accumulation is partly linked to the sea-level related changes in the size if the Patagonian source area due to the particular morphology of the Argentine shelf. We suggest that sea-level drops at the beginning of MIS 4 and MIS 2 were important for long-term dust increases, while changes in the Patagonian dust source regions primarily control the early dust decrease during the MIS 4/3 transition and Termination 1.

Dust storm from Syria- a potential new aerosol source in the E. Mediterranean- A ceilometer and synoptic study

NASA Astrophysics Data System (ADS)

Alpert, Pinhas; Egert, Smadar; Uzan, Leenes

2017-04-01

On 7 Sep 2015 an unprecedented huge dust plume approached the SE Mediterranean basin from the northeast- Syria region. According to the Israeli meteorological service it is the first time in 75 years of measurements, that a dust storm reaches Israel early September, lasts several days and dust concentrations reach values 100 times the normal (1700µg/m3). Dust storms are normally monitored in the east Mediterranean using satellites and surface PM data. Obviously, these cannot show the vertical evolution of the dust including penetration, sinking and cleaning since vertical profiles are not available. High-resolution, micro Lidar Ceilometer network is gradually established in Israel. A few instruments of this network were already operational during the dust storm. The most crucial vertical information, monitored by these Ceilometers with 10m resolution vertically, every 16s, is analyzed. The difference in the cloud-layers allow the investigation of the high altitude of 1000m dust penetration, its sinking into the complex structured 250-500m mixed layer and the gradual 3D cleaning. This finding contradicts the conventional understanding that cleaning is due to gradual descent and shows not only the vertical fluctuation during the entire event but also the vertical rise to 2000m at the end of the event. The vertical information showed that the actual event period duration was 7 days, compared to only 90 hours based on traditional detectors. Is it a new dust source in the E. Mediterranean-long and short term trends?

The Paleozoic Dust Bowl: Dust Deposition in Tropical Western Pangaea (Midcontinent U.S.) at the Terminus of the Late Paleozoic Ice Age

NASA Astrophysics Data System (ADS)

Soreghan, G. S.; Heavens, N. G.; Benison, K. C.; Soreghan, M. J.; Mahowald, N. M.; Foster, T.; Zambito, J.; Sweet, A.; Kane, M.

2012-12-01

Atmospheric dust is well recognized and studied as both an archive and agent of climate change in Earth's relatively recent past. Archives of past dust include loess deposits and dust recovered from ocean- and ice-cores. Dust remains poorly known in Earth's past prior to the Cenozoic, but is increasingly recognized in the form of paleo-loess deposits, and (epeiric) marine strata that accumulated isolated from fluvio-deltaic influx. Here, we report on the growing recognition of voluminous dust deposits preserved in the Permian record of the U.S. Midcontinent (western tropical Pangaea). Fine-grained redbeds predominate in Permian strata throughout the U.S. Midcontinent, but notably in a swath extending from Oklahoma through South Dakota. These units consist predominantly of red mudstone and siltstone in commonly massive units, but sedimentary structures and bedding that signal aqueous processes (e.g. laminations, ripples) have led most to infer deltaic or tidal deposition. The absence of channel systems to deliver the sediment, as well as the predominantly massive and laterally continuous character and the uniform fine grain size signal wind transport, implying that these units record sustained dust deposition overprinted at times by sub-aqueous deposition in lakes, including ephemeral saline and acid lakes that led to evaporite cementation. Detrital zircon geochronology indicates that much of the dust originated in the relatively distant Appalachian-Ouachita orogenic systems, which formed part of the central Pangaean mountains (CPM), the collisional zone that sutured the supercontinent. Within the Anadarko basin of Oklahoma, Permian redbeds record >2 km of predominantly dust deposition, some of the thickest dust deposits yet documented in Earth's record. Yet the tropical setting is remarkably non-uniformitarian, as much Quaternary loess occurs in mid- to high-latitude regions, commonly linked to glacial genesis. We are currently investigating with both data and modeling possible causes and consequences of this massive dust record, which may include (1) partial glacial genesis in the CPM, (2) the action of the Pangaean mega-monsoon, and (3) particularly effective dust traps in the Midcontinent region. Modeling constrains the erosivity (the effect of winds and soil moisture effects) of a range of possible climate states on dust mobilization and underscores the relative difficulty of sourcing dust directly from the Appalachian-Ouachita orogenic system under most circumstances. Combining data and modeling helps constrain the erodibility (sediment availability, coherence, etc.) of dust sources. Reconstructions of marine dust deposition to the south and the west of the Anadarko basin suggest glacial-interglacial timescale erodibility changes were similar to those seen in the Midcontinent in the last 20,000 years, when it was at a much higher latitude.

Source apportionment of PM10 and PM2.5 air pollution, and possible impacts of study characteristics in South Korea.

PubMed

Ryou, Hyoung Gon; Heo, Jongbae; Kim, Sun-Young

2018-09-01

Studies of source apportionment (SA) for particulate matter (PM) air pollution have enhanced understanding of dominant pollution sources and quantification of their contribution. Although there have been many SA studies in South Korea over the last two decades, few studies provided an integrated understanding of PM sources nationwide. The aim of this study was to summarize findings of PM SA studies of South Korea and to explore study characteristics. We selected studies that estimated sources of PM 10 and PM 2.5 performed for 2000-2017 in South Korea using Positive Matrix Factorization and Chemical Mass Balance. We reclassified the original PM sources identified in each study into seven categories: motor vehicle, secondary aerosol, soil dust, biomass/field burning, combustion/industry, natural source, and others. These seven source categories were summarized by using frequency and contribution across four regions, defined by northwest, west, southeast, and southwest regions, by PM 10 and PM 2.5 . We also computed the population-weighted mean contribution of each source category. In addition, we compared study features including sampling design, sampling and lab analysis methods, chemical components, and the inclusion of Asian dust days. In the 21 selected studies, all six PM 10 studies identified motor vehicle, soil dust, and combustion/industry, while all 15 PM 2.5 studies identified motor vehicle and soil dust. Different from the frequency, secondary aerosol produced a large contribution to both PM 10 and PM 2.5 . Motor vehicle contributed highly to both, whereas the contribution of combustion/industry was high for PM 10 . The population-weighted mean contribution was the highest for the motor vehicle and secondary aerosol sources for both PM10 and PM2.5. However, these results were based on different subsets of chemical speciation data collected at a single sampling site, commonly in metropolitan areas, with short overlap and measured by different lab analysis methods. We found that motor vehicle and secondary aerosol were the most common and influential sources for PM in South Korea. Our study, however, suggested a caution to understand SA findings from heterogeneous study features for study designs and input data. Copyright © 2018. Published by Elsevier Ltd.

Simulating Black Carbon and Dust and their Radiative Forcing in Seasonal Snow: A Case Study over North China with Field Campaign Measurements

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zhao, Chun; Hu, Zhiyuan; Qian, Yun

2014-10-30

A state-of-the-art regional model, WRF-Chem, is coupled with the SNICAR model that includes the sophisticated representation of snow metamorphism processes available for climate study. The coupled model is used to simulate the black carbon (BC) and dust concentrations and their radiative forcing in seasonal snow over North China in January-February of 2010, with extensive field measurements used to evaluate the model performance. In general, the model simulated spatial variability of BC and dust mass concentrations in the top snow layer (hereafter BCS and DSTS, respectively) are quantitatively or qualitatively consistent with observations. The model generally moderately underestimates BCS in themore » clean regions but significantly overestimates BCS in some polluted regions. Most model results fall into the uncertainty ranges of observations. The simulated BCS and DSTS are highest with >5000 ng g-1 and up to 5 mg g-1, respectively, over the source regions and reduce to <50 ng g-1 and <1 μg g-1, respectively, in the remote regions. BCS and DSTS introduce similar magnitude of radiative warming (~10 W m-2) in snowpack, which is comparable to the magnitude of surface radiative cooling due to BC and dust in the atmosphere. This study represents the first effort in using a regional modeling framework to simulate BC and dust and their direct radiative forcing in snow. Although a variety of observational datasets have been used to attribute model biases, some uncertainties in the results remain, which highlights the need for more observations, particularly concurrent measurements of atmospheric and snow aerosols and the deposition fluxes of aerosols, in future campaigns.« less

A CASE AGAINST SPINNING PAHS AS THE SOURCE OF THE ANOMALOUS MICROWAVE EMISSION

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hensley, Brandon S.; Draine, B. T.; Meisner, Aaron M., E-mail: brandon.s.hensley@jpl.nasa.gov

2016-08-10

We employ an all-sky map of the anomalous microwave emission (AME) produced by component separation of the microwave sky to study correlations between the AME and Galactic dust properties. We find that while the AME is highly correlated with all tracers of dust emission, the best predictor of the AME strength is the dust radiance. Fluctuations in the AME intensity per dust radiance are uncorrelated with fluctuations in the emission from polycyclic aromatic hydrocarbons (PAHs), casting doubt on the association between AME and PAHs. The PAH abundance is strongly correlated with the dust optical depth and dust radiance, consistent withmore » PAH destruction in low density regions. We find that the AME intensity increases with increasing radiation field strength, at variance with predictions from the spinning dust hypothesis. Finally, the temperature dependence of the AME per dust radiance disfavors the interpretation of the AME as thermal emission. A reconsideration of other AME carriers, such as ultrasmall silicates, and other emission mechanisms, such as magnetic dipole emission, is warranted.« less

Herschel observations of the Galactic H II region RCW 79

NASA Astrophysics Data System (ADS)

Liu, Hong-Li; Figueira, Miguel; Zavagno, Annie; Hill, Tracey; Schneider, Nicola; Men'shchikov, Alexander; Russeil, Delphine; Motte, Frédérique; Tigé, Jérémy; Deharveng, Lise; Anderson, Loren D.; Li, Jin-Zeng; Wu, Yuefang; Yuan, Jing-Hua; Huang, Maohai

2017-06-01

Context. Triggered star formation around H II regions could be an important process. The Galactic H II region RCW 79 is a prototypical object for triggered high-mass star formation. Aims: We aim to obtain a census of the young stellar population observed at the edges of the H II region and to determine the properties of the young sources in order to characterize the star formation processes that take place at the edges of this ionized region. Methods: We take advantage of Herschel data from the surveys HOBYS, "Evolution of Interstellar Dust", and Hi-Gal to extract compact sources. We use the algorithm getsources. We complement the Herschel data with archival 2MASS, Spitzer, and WISE data to determine the physical parameters of the sources (e.g., envelope mass, dust temperature, and luminosity) by fitting the spectral energy distribution. Results: We created the dust temperature and column density maps along with the column density probability distribution function (PDF) for the entire RCW 79 region. We obtained a sample of 50 compact sources in this region, 96% of which are situated in the ionization-compressed layer of cold and dense gas that is characterized by the column density PDF with a double-peaked lognormal distribution. The 50 sources have sizes of 0.1-0.4 pc with a typical value of 0.2 pc, temperatures of 11-26 K, envelope masses of 6-760 M⊙, densities of 0.1-44 × 105 cm-3, and luminosities of 19-12 712 L⊙. The sources are classified into 16 class 0, 19 intermediate, and 15 class I objects. Their distribution follows the evolutionary tracks in the diagram of bolometric luminosity versus envelope mass (Lbol-Menv) well. A mass threshold of 140 M⊙, determined from the Lbol-Menv diagram, yields 12 candidate massive dense cores that may form high-mass stars. The core formation efficiency (CFE) for the 8 massive condensations shows an increasing trend of the CFE with density. This suggests that the denser the condensation, the higher the fraction of its mass transformation into dense cores, as previously observed in other high-mass star-forming regions. Herschel is an ESA space observatory with science instruments provided by European-led Principal Investigator consortia and with important participation from NASA.Final reduced data and maps used in the paper (FITS format) are only available at the CDS via anonymous ftp to http://cdsarc.u-strasbg.fr (http://130.79.128.5) or via http://cdsarc.u-strasbg.fr/viz-bin/qcat?J/A+A/602/A95

Test chamber investigation of the volatilization from source materials of brominated flame retardants and their subsequent deposition to indoor dust.

PubMed

Rauert, C; Harrad, S; Stranger, M; Lazarov, B

2015-08-01

Numerous studies have reported elevated concentrations of brominated flame retardants (BFRs) in dust from indoor micro-environments. Limited information is available, however, on the pathways via which BFRs in source materials transfer to indoor dust. The most likely hypothesized pathways are (a) volatilization from the source with subsequent partitioning to dust, (b) abrasion of the treated product, transferring microscopic fibers or particles to the dust (c) direct uptake to dust via contact between source and dust. This study reports the development and application of an in-house test chamber for investigating BFR volatilization from source materials and subsequent partitioning to dust. The performance of the chamber was evaluated against that of a commercially available chamber, and inherent issues with such chambers were investigated, such as loss due to sorption of BFRs to chamber surfaces (so-called sink effects). The partitioning of polybrominated diphenyl ethers to dust, post-volatilization from an artificial source was demonstrated, while analysis in the test chamber of a fabric curtain treated with the hexabromocyclododecane formulation, resulted in dust concentrations exceeding substantially those detected in the dust pre-experiment. These results provide the first experimental evidence of BFR volatilization followed by deposition to dust. Brominated flame retardants (BFRs) are ubiquitous in indoor air and dust, leading to human exposure and resultant concerns about their adverse impact on health. Indoor dust has been demonstrated to constitute an important vector of human exposure to BFRs, especially for toddlers. Despite the greater importance of dust contamination in the context of human exposure to BFRs, the mechanisms via which BFRs transfer from source materials to dust have hitherto been subject to only limited research. In this study, a test chamber is utilized to simulate the migration of BFRs to dust via volatilization from source materials and subsequent deposition to dust. © 2014 John Wiley & Sons A/S. Published by John Wiley & Sons Ltd.

Dust storm in Alaska

NASA Image and Video Library

2013-11-18

Dust storm in Alaska captured by Aqua/MODIS on Nov. 17, 2013 at 21:45 UTC. When glaciers grind against underlying bedrock, they produce a silty powder with grains finer than sand. Geologists call it “glacial flour” or “rock flour.” This iron- and feldspar-rich substance often finds its ways into rivers and lakes, coloring the water brown, grey, or aqua. When river or lake levels are low, the flour accumulates on drying riverbanks and deltas, leaving raw material for winds to lift into the air and create plumes of dust. Scientists are monitoring Arctic dust for a number of reasons. Dust storms can reduce visibility enough to disrupt air travel, and they can pose health hazards to people on the ground. Dust is also a key source of iron for phytoplankton in regional waters. Finally, there is the possibility that dust events are becoming more frequent and severe due to ongoing recession of glaciers in coastal Alaska. To read more about dust storm in this region go to: earthobservatory.nasa.gov/IOTD/view.php?id=79518 Credit: NASA/GSFC/Jeff Schmaltz/MODIS Land Rapid Response Team NASA image use policy. NASA Goddard Space Flight Center enables NASA’s mission through four scientific endeavors: Earth Science, Heliophysics, Solar System Exploration, and Astrophysics. Goddard plays a leading role in NASA’s accomplishments by contributing compelling scientific knowledge to advance the Agency’s mission. Follow us on Twitter Like us on Facebook Find us on Instagram

Modern Dust Deposition and Dissolved Iron Residence Times in the Eastern Tropical Pacific Ocean

NASA Astrophysics Data System (ADS)

Vivancos, S. M.; Anderson, R. F.; Pavia, F. J.; Fleisher, M. Q.; Lu, Y.; Zhang, P.; Cheng, H.; Edwards, R. L.

2016-02-01

We use dissolved 230Th and 232Th data along the U.S. GEOTRACES Equatorial Pacific Zonal Transect (EPZT) from Peru to Tahiti to quantify dust input to the region. Dust in the global oceans is a mineral ballast that helps carry organic matter to depth, a reactive particle surface that scavenges trace metals such as Th and Pa from the water column, and through its dissolution dust provides essential micronutrients, such as iron, that stimulate productivity. When integrating Th inventories from the sea surface to 500 meters water depth (Hayes et al., Earth Planet. Sci. Lett., 383 (2013) 16-25), we find that dust fluxes along the EPZT are an order of magnitude lower (0.18-1.61 g/m2/yr) than along the U.S. GEOTRACES Atlantic Transect (Mauritania to Bermuda; 3.22 to 10.56 g/m2/yr). Dust fluxes decrease with distance away from the dust source (i.e., the continents). Using an Fe/Th ratio of 2660 g/g for dust and assuming a Fe/Th solubility ratio of 1.0 (Hayes et al., Geochim. Cosmochim. Acta, 169 (2015) 1-16), we calculate a dissolved iron flux of 12.06 to 109.88 µmol/m2/yr to the EPZT region. Utilizing dissolved iron data along the EPZT (Resing et al., Nature, 523 (2015) 200-203), we calculate a dissolved iron residence time integrated from the sea surface to 500 meters water depth of 4 to 11 years.

Signals of pollution revealed by trace elements in recent snow from mountain glaciers at the Qinghai-Tibetan plateau.

PubMed

Li, Yuefang; Li, Zhen; Cozzi, Giulio; Turetta, Clara; Barbante, Carlo; Huang, Ju; Xiong, Longfei

2018-06-01

In order to extract pollution signal of trace elements (TEs) in glacier snow at the Qinghai-Tibetan plateau of China by human activities, concentrations of 18 TEs (Al, Ti, Fe, Rb, Sr, Ba, V, Cr, Mn, Li, Cu, Co, Mo, Cs, Sb, Pb, Tl, and U), 14 rare earth elements (La, Ce, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, and Lu), Y and Th in digested snow samples from five glaciers in April-May 2013 before monsoon season were measured. Results shown that higher TEs concentrations were found in glaciers at the northern plateau while lower concentrations in glaciers at the central and southern plateau. Discussion revealed that EF values calculated from elements with mass fraction <30% such as Ti and Al, etc in traditional acid leached samples, will overestimate at least 4.6 times the contribution of other sources than dust for TEs such as Sb, Sr, As, Cu and Pb etc. Analysis indicated that most TEs mainly originated from dust sources, whereas Pb, Cu, Mo and Sb showed occasionally significant contributions from polluted sources in three snow pits and the GRHK surface snow samples. The pollution probably originated from mining and smelting, road transport emissions on the plateau and some regions outside of the plateau. Dust provenance tracing results based on REEs indicated that Taklimakan Desert, Qaidam Basin, and Tibetan surface soil were the potential dust sources for the studied glaciers, while the Indian Thar Desert was an occasional dust sources for YZF,XDKMD and GRHK snow samples. Copyright © 2018 Elsevier Ltd. All rights reserved.

The ALMA-PILS survey: 3D modeling of the envelope, disks and dust filament of IRAS 16293-2422

NASA Astrophysics Data System (ADS)

Jacobsen, S. K.; Jørgensen, J. K.; van der Wiel, M. H. D.; Calcutt, H.; Bourke, T. L.; Brinch, C.; Coutens, A.; Drozdovskaya, M. N.; Kristensen, L. E.; Müller, H. S. P.; Wampfler, S. F.

2018-04-01

Context. The Class 0 protostellar binary IRAS 16293-2422 is an interesting target for (sub)millimeter observations due to, both, the rich chemistry toward the two main components of the binary and its complex morphology. Its proximity to Earth allows the study of its physical and chemical structure on solar system scales using high angular resolution observations. Such data reveal a complex morphology that cannot be accounted for in traditional, spherical 1D models of the envelope. Aims: The purpose of this paper is to study the environment of the two components of the binary through 3D radiative transfer modeling and to compare with data from the Atacama Large Millimeter/submillimeter Array. Such comparisons can be used to constrain the protoplanetary disk structures, the luminosities of the two components of the binary and the chemistry of simple species. Methods: We present 13CO, C17O and C18O J = 3-2 observations from the ALMA Protostellar Interferometric Line Survey (PILS), together with a qualitative study of the dust and gas density distribution of IRAS 16293-2422. A 3D dust and gas model including disks and a dust filament between the two protostars is constructed which qualitatively reproduces the dust continuum and gas line emission. Results: Radiative transfer modeling in our sampled parameter space suggests that, while the disk around source A could not be constrained, the disk around source B has to be vertically extended. This puffed-up structure can be obtained with both a protoplanetary disk model with an unexpectedly high scale-height and with the density solution from an infalling, rotating collapse. Combined constraints on our 3D model, from observed dust continuum and CO isotopologue emission between the sources, corroborate that source A should be at least six times more luminous than source B. We also demonstrate that the volume of high-temperature regions where complex organic molecules arise is sensitive to whether or not the total luminosity is in a single radiation source or distributed into two sources, affecting the interpretation of earlier chemical modeling efforts of the IRAS 16293-2422 hot corino which used a single-source approximation. Conclusions: Radiative transfer modeling of source A and B, with the density solution of an infalling, rotating collapse or a protoplanetary disk model, can match the constraints for the disk-like emission around source A and B from the observed dust continuum and CO isotopologue gas emission. If a protoplanetary disk model is used around source B, it has to have an unusually high scale-height in order to reach the dust continuum peak emission value, while fulfilling the other observational constraints. Our 3D model requires source A to be much more luminous than source B; LA 18 L⊙ and LB 3 L⊙.

Relative Contributions of the Saharan and Sahelian Sources to the Atmospheric Dust Load Over the North Atlantic

NASA Technical Reports Server (NTRS)

Ginoux, Paul; Chin, M.; Torres, O.; Prospero, J.; Dubovik, O.; Holben, B.; Einaudi, Franco (Technical Monitor)

2000-01-01

It has long been recognized that Saharan desert is the major source for long range transport of mineral dust over the Atlantic. The contribution from other natural sources to the dust load over the Atlantic has generally been ignored in previous model studies or been replaced by anthropogenically disturbed soil emissions. Recently, Prospero et.at. have identified the major dust sources over the Earth using TOMS aerosol index. They showed that these sources correspond to dry lakes with layers of sediment deposed in the late Holocene or Pleistocene. One of the most active of these sources seem to be the Bodele depression. Chiapello et al. have analyzed the mineralogical composition of dust on the West coast of Africa. They found that Sahelian dust events are the most intense but are less frequent than Saharan plumes. This suggests that the Bodele depression could contribute significantly to the dust load over the Atlantic. The relative contribution of the Sahel and Sahara dust sources is of importance for marine biogeochemistry or atmospheric radiation, because each source has a distinct mineralogical composition. We present here a model study of the relative contributions of Sahara and Sahel sources to the atmospheric dust aerosols over the North Atlantic. The Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model is used to simulate dust distribution in 1996-1997. Dust particles are labeled depending on their sources. In this presentation, we will present the comparison between the model results and observations from ground based measurements (dust concentration, optical thickness and size distribution) and satellite data (TOMS aerosol index). The relative contribution of each source will then be analyzed spatially and temporally.

Do some of the sub-micrometer cosmic dust particles come from the sun.

NASA Technical Reports Server (NTRS)

Hemenway, C. L.; Erkes, J. W.; Greenberg, J. M.; Hallgren, D. S.; Schmalberger, D. C.

1973-01-01

Studies of cosmic dust particles collected at altitudes of 80 to 120 km over White Sands, New Mexico, and at times of noctilucent clouds over Kiruna, Sweden, indicate that an anomalously high atomic weight contribution is present within those particles collected at Kiruna. The elements observed are inconsistent with an origin due to atomic bomb fallout, meteoroidal crumbling, lunar ejecta, or comets. Many of these heavy elements may be stable in particulate form at the relatively high temperatures found in the coolest regions of the solar atmosphere. Some implications of the sun as the source of a significant component of cosmic dust are discussed.

Multi-Decadal Aerosol Variations from 1980 to 2009: A Perspective from Observations and a Global Model

NASA Technical Reports Server (NTRS)

Chin, Mian; Diehl, T.; Tan, Q.; Prospero, J. M.; Kahn, R. A.; Remer, L. A.; Yu, H.; Sayer, A. M.; Bian, H.; Geogdzhayev, I. V.;

Sources, Sinks, and Transatlantic Transport of North African Dust Aerosol: A Multimodel Analysis and Comparison With Remote Sensing Data

NASA Technical Reports Server (NTRS)

Kim, Dongchul; Chin, Mian; Yu, Hongbin; Diehl, Thomas; Tan, Qian; Kahn, Ralph A.; Tsigaridis, Kostas; Bauer, Susanne E.; Takemura, Toshihiko; Pozzoli, Luca;

Modeling the emission, transport and deposition of contaminated dust from a mine tailing site.

PubMed

Stovern, Michael; Betterton, Eric A; Sáez, A Eduardo; Villar, Omar Ignacio Felix; Rine, Kyle P; Russell, Mackenzie R; King, Matt

2014-01-01

Mining operations are potential sources of airborne particulate metal and metalloid contaminants through both direct smelter emissions and wind erosion of mine tailings. The warmer, drier conditions predicted for the Southwestern US by climate models may make contaminated atmospheric dust and aerosols increasingly important, due to potential deleterious effects on human health and ecology. Dust emissions and dispersion of contaminants from the Iron King Mine tailings in Dewey-Humboldt, Arizona, a Superfund site, are currently being investigated through in situ field measurements and computational fluid dynamics modeling. These tailings are significantly contaminated with lead and arsenic with an average soil concentration of 1616 and 1420 ppm, respectively. Similar levels of these contaminants have also been measured in soil samples taken from the area surrounding the mine tailings. Using a computational fluid dynamics model, we have been able to model dust transport from the mine tailings to the surrounding region. The model includes a distributed Eulerian model to simulate fine aerosol transport and a Lagrangian approach to model fate and transport of larger particles. In order to improve the accuracy of the dust transport simulations both regional topographical features and local weather patterns have been incorporated into the model simulations.

Synoptic characteristics of dust over the southwest of Iran

NASA Astrophysics Data System (ADS)

Katiraie-Boroujerdy, P.; Ghahri, F.; Ranjbar Saadatabadi, A.

2012-12-01

Iran is frequently affected by dust events because it is located in arid and semiarid belt of the world. As Khozestan province is in the vicinity of large deserts and also due to especial atmospheric conditions the frequency of dust in this area is increased in the recent years. Therefore it has the destructive affect on the healthcare, economy, social and etc. The study is based on the, sea level, 850 mb and 500 mb weather charts, surface wind field and observations weather data during the period of 1968-2008. By numerical simulation with WRF modeling it has tried to high light provide an answer to how this event produced and reached to Ahwaz. It has been shown in this 40 years, dust events by high strength and frequency occur in July in Ahwaz. Synoptic patterns revealed that for making sever dust event Persian Gulf thermal trough extends to the north west of Iraq and European ridge extends over the Black sea and large part of the Turkey by passing waves of middle level Mediterranean trough from northwest of Iraq and east of Syria. Numerical simulation shows strong surface flow over source regions in northwest of Iraq and east of Syria, creation westerly low level jet in low-lying areas and the increase in friction velocity in the source regions. In the deserts of Iraq and north east of Syria increase in friction velocity to its highest value (approx 0.6 m/s) causes reduction in visibility and by decrease to lowest value (approx 0.4 m/s) visibility reaches up to 600 meters in Ahwaz.

Impact of Surface Roughness and Soil Texture on Mineral Dust Emission Fluxes Modeling

NASA Technical Reports Server (NTRS)

Menut, Laurent; Perez, Carlos; Haustein, Karsten; Bessagnet, Bertrand; Prigent, Catherine; Alfaro, Stephane

2013-01-01

Dust production models (DPM) used to estimate vertical fluxes of mineral dust aerosols over arid regions need accurate data on soil and surface properties. The Laboratoire Inter-Universitaire des Systemes Atmospheriques (LISA) data set was developed for Northern Africa, the Middle East, and East Asia. This regional data set was built through dedicated field campaigns and include, among others, the aerodynamic roughness length, the smooth roughness length of the erodible fraction of the surface, and the dry (undisturbed) soil size distribution. Recently, satellite-derived roughness length and high-resolution soil texture data sets at the global scale have emerged and provide the opportunity for the use of advanced schemes in global models. This paper analyzes the behavior of the ERS satellite-derived global roughness length and the State Soil Geographic data base-Food and Agriculture Organization of the United Nations (STATSGO-FAO) soil texture data set (based on wet techniques) using an advanced DPM in comparison to the LISA data set over Northern Africa and the Middle East. We explore the sensitivity of the drag partition scheme (a critical component of the DPM) and of the dust vertical fluxes (intensity and spatial patterns) to the roughness length and soil texture data sets. We also compare the use of the drag partition scheme to a widely used preferential source approach in global models. Idealized experiments with prescribed wind speeds show that the ERS and STATSGO-FAO data sets provide realistic spatial patterns of dust emission and friction velocity thresholds in the region. Finally, we evaluate a dust transport model for the period of March to July 2011 with observed aerosol optical depths from Aerosol Robotic Network sites. Results show that ERS and STATSGO-FAO provide realistic simulations in the region.

Some Coolness on Martian Global Warming and Reflections on the Role of Surface Dust

NASA Astrophysics Data System (ADS)

Richardson, M. I.; Vasavada, A. R.

2007-12-01

Recent comparisons of global snap-shots of Mars' surface taken by the Viking and Mars Global Surveyor (MGS) cameras have been used to suggest that Mars has darkened, and hence has warmed, between the 1970's and 1990's. While this conclusion is not supported by more quantitative analysis of albedo data, the idea of Martian darkening and warming has found its way into the terrestrial climate change debate. Through blogs and other opinion pieces it has been used, both amusingly and disturbingly, to argue that Mars' apparent natural warming should alleviate our concerns about anthropomorphic climate change on Earth. Relating planetary research results to terrestrial analogs is instructive and promotes public understanding, but this example provides a cautionary tale of misinterpretation in this age of politicized science. The dust cycle is the dominant short-term component of the Martian climate. The atmosphere is strongly forced via dust's modification of atmospheric radiative heating rates, while dust loading displays dramatic interannual variability, from background opacity to aperiodic global dust storms. Until recently, the atmospheric component of the dust cycle was better documented than the surface component (which on Mars can be gauged via albedo). But now thanks to the combination of regional imaging, spot thermal infrared spectra, and spot short-wavelength photometry sampled at synoptic time and length scales by MGS, a rich new view of the relationship between specific meteorological phenomena and the patterns of surface dust is emerging. Seasonal cap winds, local, regional, and global dust storms, and monsoonal circulations all redistribute surface dust on large spatial scales, while dust devils are surprisingly shown to be insignificant. Rapid and widespread albedo modification is accomplished by storms that darken relatively bright regions through dust removal, and deposit dust upon largely dust free areas, brightening them. (It is not possible with existing data to infer dust deposition or erosion in perennially dusty areas.) However, most of the dust deposited on darker regions is removed within one Martian year. This rapid cleaning suggests that darker areas retain their dust-free albedo over decadal time scales because any dust deposited there can be eroded at commonly experienced wind speeds. Bright regions recover more slowly, sometimes requiring several martian years. The depletion of these dust sources in some years may play an important role in the interannual variability in dust storm occurrence and intensity by introducing a multiyear "memory" into the system. The observation of the 2001 global storm and its wake allows predictions to be made for the recovery following the 2007 global storm: the southern hemisphere should retain a transient brightening until after the seasonal cap has advanced and retreated. The MGS data show that albedo is a dynamic and evolving meteorologically and climatologically active variable, not a static boundary condition. Overall, the major story that albedo has to tell is one of major dust storms and recovery from them - not of secular changes - and that the changes are mostly cyclic such that surfaces tend to return to their pre-storm albedos. We speculate that this system of fine balances is dynamically controlled, such that interannual occurrence of dust storms and the partial dust coating of the surface should be robust against the expected large changes of orbital parameters throughout Martian geological history.

Lidar Measurements of the Vertical Distribution of Aerosol Optical and Physical Properties over Central Asia

DOE PAGES

Chen, Boris B.; Sverdlik, Leonid G.; Imashev, Sanjar A.; ...

2013-01-01

The vertical structure of aerosol optical and physical properties was measured by Lidar in Eastern Kyrgyzstan, Central Asia, from June 2008 to May 2009. Lidar measurements were supplemented with surface-based measurements of PM 2.5 and PM 10 mass and chemical composition in both size fractions. Dust transported into the region is common, being detected 33% of the time. The maximum frequency occurred in the spring of 2009. Dust transported to Central Asia comes from regional sources, for example, Taklimakan desert and Aral Sea basin, and from long-range transport, for example, deserts of Arabia, Northeast Africa, Iran, and Pakistan. Regional sourcesmore » are characterized by pollution transport with maximum values of coarse particles within the planetary boundary layer, aerosol optical thickness, extinction coefficient, integral coefficient of aerosol backscatter, and minimum values of the Ångström exponent. Pollution associated with air masses transported over long distances has different characteristics during autumn, winter, and spring. During winter, dust emissions were low resulting in high values of the Ångström exponent (about 0.51) and the fine particle mass fraction (64%). Dust storms were more frequent during spring with an increase in coarse dust particles in comparison to winter. The aerosol vertical profiles can be used to lower uncertainty in estimating radiative forcing.« less

Sensitivity of desert dust emission modelling to horizontal resolution: the example of the Bodélé Depression

NASA Astrophysics Data System (ADS)

Bouet, Christel; Cautenet, Guy; Marticorena, Béatrice; Bergametti, Gilles; Minvielle, Fanny; Schmechtig, Catherine; Laurent, Benoit

2010-05-01

Atmospheric aerosols are known to play an important role in the Earth's climate system. However, the quantification of aerosol radiative impact on the Earth's radiative budget is very complex because of the high variability in space and time of aerosol mass and particle number concentrations, and optical properties as well. In many regions, like in desert regions, dust is the largest contribution to aerosol optical thickness [Tegen et al., 1997]. Consequently, it appears fundamental to well represent mineral dust emissions to reduce uncertainties concerning aerosol radiative impact on the Earth's radiative budget. Recently, several studies (e.g. Prospero et al. [2002]) underlined that the Bodélé depression, in northern Chad, is probably the most important source of mineral dust in the world. However many models fail in simulating these large dust emissions. Indeed, dust emission is a threshold phenomenon mainly driven by the intensity of surface wind velocity. Realistic estimates of dust emissions then rely on the quality and accuracy of the surface wind fields. Koren and Kaufman [2004] showed that the reanalysis data (NCEP), which can be used as input data in numerical models, underestimates surface wind velocity in the Bodélé Depression by up to 50%. Such an uncertainty on surface wind velocity cannot allow an accurate simulation of the dust emission. In mesoscale meteorological models, global reanalysis datasets are used to initialize and laterally nudge the models that compute meteorological parameters (like wind velocity) with a finer spatial and temporal resolutions. The question arises concerning the precision of the wind speeds calculated by these models. Using the Regional Atmospheric Modeling System (RAMS, Cotton et al. [2003]) coupled online with the dust production model developed by Marticorena and Bergametti [1995] and recently improved by Laurent et al. [2008] for Africa, the influence of the horizontal resolution of the mesoscale meteorological model on the simulation of dust emission in the Bodélé Depression is investigated. A one year simulation is run in order to test the capability of the model to represent the pronounced seasonal cycle of dust emission in this region. Routine measurements from meteorological stations as well as satellite imagery are used to evaluate the accuracy of the simulations.

Laboratory Investigations of the Physical and Optical Properties of the Analogs of Individual Cosmic Dust Grains

NASA Technical Reports Server (NTRS)

Abbas, M. M.; Tankosic, D.; Craven, P. D.; Spann, J. F.; LeClair, A.; West, E. A.

2005-01-01

Microdsub-micron size cosmic dust grains play an important role in the physical and dynamical process in the galaxy, the interstellar medium, and the interplanetary and planetary environments. The dust grains in various astrophysical environments are generally charged by a variety of mechanisms that include collisional process with electrons and ions, and photoelectric emissions with UV radiation. The photoelectric emission process is believed to be the dominant process in many astrophysical environments with nearby UV sources, such as the interstellar medium, diffuse clouds, the outer regions of the dense molecular clouds, interplanetary medium, dust in planetary environments and rings, cometary tails, etc. Also, the processes and mechanisms involved in the rotation and alignment of interstellar dust grains are of great interest in view of the polarization of observed starlight as a probe for evaluation of the galactic magnetic field.

Emission, transport, and radiative effects of mineral dust from the Taklimakan and Gobi deserts: comparison of measurements and model results

NASA Astrophysics Data System (ADS)

Chen, Siyu; Huang, Jianping; Kang, Litai; Wang, Hao; Ma, Xiaojun; He, Yongli; Yuan, Tiangang; Yang, Ben; Huang, Zhongwei; Zhang, Guolong

2017-02-01

The Weather Research and Forecasting Model with chemistry (WRF-Chem model) was used to investigate a typical dust storm event that occurred from 18 to 23 March 2010 and swept across almost all of China, Japan, and Korea. The spatial and temporal variations in dust aerosols and the meteorological conditions over East Asia were well reproduced by the WRF-Chem model. The simulation results were used to further investigate the details of processes related to dust emission, long-range transport, and radiative effects of dust aerosols over the Taklimakan Desert (TD) and Gobi Desert (GD). The results indicated that weather conditions, topography, and surface types in dust source regions may influence dust emission, uplift height, and transport at the regional scale. The GD was located in the warm zone in advance of the cold front in this case. Rapidly warming surface temperatures and cold air advection at high levels caused strong instability in the atmosphere, which strengthened the downward momentum transported from the middle and low troposphere and caused strong surface winds. Moreover, the GD is located in a relatively flat, high-altitude region influenced by the confluence of the northern and southern westerly jets. Therefore, the GD dust particles were easily lofted to 4 km and were the primary contributor to the dust concentration over East Asia. In the dust budget analysis, the dust emission flux over the TD was 27.2 ± 4.1 µg m-2 s-1, which was similar to that over the GD (29 ± 3.6 µg m-2 s-1). However, the transport contribution of the TD dust (up to 0.8 ton d-1) to the dust sink was much smaller than that of the GD dust (up to 3.7 ton d-1) because of the complex terrain and the prevailing wind in the TD. Notably, a small amount of the TD dust (PM2.5 dust concentration of approximately 8.7 µg m-3) was lofted to above 5 km and transported over greater distances under the influence of the westerly jets. Moreover, the direct radiative forcing induced by dust was estimated to be -3 and -7 W m-2 at the top of the atmosphere, -8 and -10 W m-2 at the surface, and +5 and +3 W m-2 in the atmosphere over the TD and GD, respectively. This study provides confidence for further understanding the climate effects of the GD dust.

A Model for Saharan Dust Transport.

NASA Astrophysics Data System (ADS)

D'Almeida, Guillaume A.

1986-07-01

In this paper the source strength and the deposition rate of the dust emerging from the Sahara are assessed. For this purpose a multichannel sunphotometer has been developed and a turbidity network covering 11 stations has been set up in the Sahara, in the Sahel region and the surrounding southern area for a duration of about two years. A correlation analysis connecting observed aerosol turbidity parameters and mineral dust mass concentration has been performed during a four-week field campaign in Agadez (Niger). An appropriate box model including the aerosol turbidity parameters, actual wind field data of the source regions, the general circulation pattern over Africa and dry and wet deposition reveals a total mass production of about 630 × 106 and 710 × 106 t yr1 for all suspended particulate matter, 80 × 106 and 90 × 106 t yr1 for aerosol particles smaller than 5 m radius for the years 1981 and 1982 respectively. About 60% of the mass moves southward to the Gulf of Guinea, 28% westward to the equatorial North Atlantic Ocean and 12% northward to Europe. A considerable part is deposited in the Atlantic Ocean and the Mediterranean forming deep-sea sediments.

Synoptic conditions favouring the occurrence of dust transport from Africa toward Sardinia Island.

NASA Astrophysics Data System (ADS)

Canu, Annalisa; Pellizzaro, Grazia; Pintus, Gabriella; Duce, Pierpaolo

2016-04-01

Dust events that reach Italy have usually origin in the Sahara and Sahel regions (north-western part of Africa), which represent the dust sources nearest to Italy. In those regions the dust-lifting activity occurs in a remarkable way. Every dust event is different from the others; in fact dust transport and dust concentration in the air can vary remarkably depending on the synoptic situation. In Sardinia, dust events are more frequent in the May-November period, but they can also take place in the December-April period. The main aim of this work was to describe dust outbreaks in Sardinia and to identify the main meteorological scenarios that originate the transport of dust towards the central and western Mediterranean Basin. The evaluation of the geographical dispersion of Saharan dust was performed by using MODIS satellite data and Meteosat imagery combined with SKIRON forecasting model. The origin and the trajectory of the dust carried by winds towards Italy were inferred by the NOAA HYSPLIT model (Hybrid Single Particle Lagrangian Integrated Trajectory Model). In addition, PM10 (particulate matter with a diameter of less than 10 μm) and meteorological data registered by the ARPAS (Regional Environmental Protection Agency of Sardinia) monitoring stations were used to highlight the arrival of African air masses in Sardinia. The study was carried out during the 2014. A total of five events occurred during the year (two in spring and three in autumn) were analyzed. The origin of air masses loaded with dust from North Africa was confirmed by satellite imagery and 3-days air mass backward trajectories calculated by the NOAA HYSPLIT model. The analysis of the PM10 daily pattern registered at northern and southern Sardinia sites showed a rising of values during the dust event. The arrival of air masses from Africa caused the daily mean air temperature to rise whereas relative humidity values decreased. Finally, the results showed that all the event analyzed were characterized by a low-pressure system over the Iberian Peninsula that extended towards Morocco and by the associated high-pressure system over the North-East Africa (Algeria, Tunisia and Libya) and Sicily. This synoptic structure (low pressure over North-Western Africa) forced the dusty air masses towards the Mediterranean basin, favouring the transport of African air masses towards the Sardinia island.

Composition and Sources of Fine and Coarse Particles Collected during 2002–2010 in Boston, MA

PubMed Central

Masri, Shahir; Kang, Choong-Min; Koutrakis, Petros

2016-01-01

Identifying the sources, composition, and temporal variability of fine (PM2.5) and coarse (PM2.5-10) particles is a crucial component in understanding PM toxicity and establishing proper PM regulations. In this study, a Harvard Impactor was used to collect daily integrated fine and coarse particle samples every third day for nine years at a single site in Boston, MA. A total of 1,960 filters were analyzed for elements, black carbon (BC), and total PM mass. Positive Matrix Factorization (PMF) was used to identify source types and quantify their contributions to ambient PM2.5 and PM2.5-10. BC and 17 elements were identified as the main constituents in our samples. Results showed that BC, S, and Pb were associated exclusively with the fine particle mode, while 84% of V and 79% of Ni were associated with this mode. Elements mostly found in the coarse mode, over 80%, included Ca, Mn (road dust), and Cl (sea salt). PMF identified six source types for PM2.5 and three source types for PM2.5-10. Source types for PM2.5 included regional pollution, motor vehicles, sea salt, crustal/road dust, oil combustion, and wood burning. Regional pollution contributed the most, accounting for 48% of total PM2.5 mass, followed by motor vehicles (21%) and wood burning (19%). Source types for PM2.5-10 included crustal/road dust (62%), motor vehicles (22%), and sea salt (16%). A linear decrease in PM concentrations with time was observed for both fine (−5.2%/yr) and coarse (−3.6%/yr) particles. The fine-mode trend was mostly related to oil combustion and regional pollution contributions. Average PM2.5 concentrations peaked in summer (10.4 μg/m3) while PM2.5-10 concentrations were lower and demonstrated little seasonal variability. The findings of this study show that PM25 is decreasing more sharply than PM2.5-10 over time. This suggests the increasing importance of PM2.5-10 and traffic-related sources for PM exposure and future policies. PMID:25947125

Effects of two Asian sand dusts transported from the dust source regions of Inner Mongolia and northeast China on murine lung eosinophilia.

PubMed

He, Miao; Ichinose, Takamichi; Song, Yuan; Yoshida, Yasuhiro; Arashidani, Keiichi; Yoshida, Seiichi; Liu, Boying; Nishikawa, Masataka; Takano, Hirohisa; Sun, Guifan

2013-11-01

The quality and quantity of toxic materials adsorbed onto Asian sand dust (ASD) are different based on dust source regions and passage routes. The aggravating effects of two ASDs (ASD1 and ASD2) transported from the source regions of Inner Mongolia and northeast China on lung eosinophilia were compared to clarify the role of toxic materials in ASD. The ASDs contained different amounts of lipopolysaccharides (LPS) and β-glucan (ASD1ASD2). CD-1 mice were instilled intratracheally with ASD1, ASD2 and/or ovalbumin (OVA) four times at 2-week intervals. ASD1 and ASD2 enhanced eosinophil recruitment induced by OVA in the submucosa of the airway, with goblet cell proliferation in the bronchial epithelium. ASD1 and ASD2 synergistically increased OVA-induced eosinophil-relevant cytokines interleukin-5 (IL-5), IL-13 (ASD1ASD2) in bronchoalveolar lavage fluid. ASD2 aggravating effects on lung eosinophilia were greater than ASD1. The role of LPS and β-glucan in ASD2 on the production of pro-inflammatory mediators was assessed using in vitro bone marrow-derived macrophages (BMDMs) from wild type, Toll-like receptor 2-deficient (TLR2-/-), TLR4-/-, and MyD88-/- mice (on Balb/c background). ASD2-stimulated TLR2-/- BMDMs enhanced IL-6, IL-12, TNF-α, MCP-1 and MIP-1α secretion compared with ASD2-stimulated TLR4-/- BMDMs. Protein expression from ASD2-stimulated MyD88-/- BMDM were very low or undetectable. The in vitro results indicate that lung eosinophilia caused by ASD is TLR4 dependent. Therefore, the aggravation of OVA-related lung eosinophilia by ASD may be dependent on toxic substances derived from microbes, such as LPS, rather than SiO2. © 2013. Published by Elsevier Inc. All rights reserved.

[Geochemical characteristics and sources of atmospheric particulates in Shanghai during dust storm event].

PubMed

Qian, Peng; Zheng, Xiang-min; Zhou, Li-min

2013-05-01

Atmospheric particulates were sampled from three sampling sites of Putuo, Minhang and Qingpu Districts in Shanghai between Oct. , 2009 and Oct. , 2010. In addition, particulate samples were also collected from Nantong, Zhengzhou, Xi'an, and Beijing city where dust storm dust transported along during spring. Element compositions of atmospheric particulates were determined by XRF and ICP-MS. The concentrations of major and trace elements in atmospheric particulates from Putuo, Minhang and Qingpu Districts were similar, indicating their common source. The UCC standardization distribution map showed that the major element composition of dust storm samples was similar to that of loess in northwestern China, indicating that the dust storm dust was mainly derived from Western desert and partly from local area. The REE partition patterns of dust storm dusts among different cities along dust transport route were similar to each other, as well as to those of northern loess, which indicates that the dust storm samples may have the same material source as loess, which mainly comes from crust material. However, the REE partition patterns of non-dust storm particulates were different among the studied cities, and different from those of loess, which suggests that the non-dust storm samples may be mixed with non-crust source material, which is different from dust storm dust and loess. The major element composition and REE partition pattern are effective indicators for source tracing of dust storm dust.

Black carbon and mineral dust in snow cover on the Tibetan Plateau

NASA Astrophysics Data System (ADS)

Zhang, Yulan; Kang, Shichang; Sprenger, Michael; Cong, Zhiyuan; Gao, Tanguang; Li, Chaoliu; Tao, Shu; Li, Xiaofei; Zhong, Xinyue; Xu, Min; Meng, Wenjun; Neupane, Bigyan; Qin, Xiang; Sillanpää, Mika

2018-02-01

Snow cover plays a key role for sustaining ecology and society in mountainous regions. Light-absorbing particulates (including black carbon, organic carbon, and mineral dust) deposited on snow can reduce surface albedo and contribute to the near-worldwide melting of snow and ice. This study focused on understanding the role of black carbon and other water-insoluble light-absorbing particulates in the snow cover of the Tibetan Plateau (TP). The results found that the black carbon, organic carbon, and dust concentrations in snow cover generally ranged from 202 to 17 468 ng g-1, 491 to 13 880 ng g-1, and 22 to 846 µg g-1, respectively, with higher concentrations in the central to northern areas of the TP. Back trajectory analysis suggested that the northern TP was influenced mainly by air masses from Central Asia with some Eurasian influence, and air masses in the central and Himalayan region originated mainly from Central and South Asia. The relative biomass-burning-sourced black carbon contributions decreased from ˜ 50 % in the southern TP to ˜ 30 % in the northern TP. The relative contribution of black carbon and dust to snow albedo reduction reached approximately 37 and 15 %, respectively. The effect of black carbon and dust reduced the snow cover duration by 3.1 ± 0.1 to 4.4 ± 0.2 days. Meanwhile, the black carbon and dust had important implications for snowmelt water loss over the TP. The findings indicate that the impacts of black carbon and mineral dust need to be properly accounted for in future regional climate projections, particularly in the high-altitude cryosphere.

Satellite Monitoring of Asian Dust Storms from SeaWiFS and MODIS: Source, Pathway, and Interannual Variability

NASA Astrophysics Data System (ADS)

Hsu, N.; Tsay, S.; Jeong, M.; Holben, B.

2006-12-01

Among the many components that contribute to air pollution, airborne mineral dust plays an important role due to its biogeochemical impact on the ecosystem and its radiative-forcing effect on the climate system. In East Asia, dust storms frequently accompany the cold and dry air masses that occur as part of spring-time cold front systems. China's capital, Beijing, and other large cities are on the primary pathway of these dust storm plumes, and their passage over such popu-lation centers causes flight delays, pushes grit through windows and doors, and forces people indoors. Furthermore, during the spring these anthropogenic and natural air pollutants, once generated over the source regions, can be transported out of the boundary layer into the free troposphere and can travel thousands of kilometers across the Pacific into the United States and beyond. In this paper, we will demonstrate the capability of a new satellite algorithm to retrieve aerosol optical thickness and single scattering albedo over bright-reflecting surfaces such as urban areas and deserts. Such retrievals have been dif-ficult to perform using previously available algorithms that use wavelengths from the mid-visible to the near IR because they have trouble separating the aerosol signal from the contribution due to the bright surface reflectance. The new algorithm, called Deep Blue, utilizes blue-wavelength measurements from instruments such as SeaWiFS and MODIS to infer the properties of aerosols, since the surface reflectance over land in the blue part of the spectrum is much lower than for longer wavelength channels. We have validated the satellite retrieved aerosol optical thickness with data from AERONET sunphotometers over desert and semi-desert regions. The compari-sons show reasonable agreements between these two. These new satellite prod-ucts will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from SeaWiFS and MODIS-like instruments. The multiyear satellite measurements since 1998 from SeaWiFS will be utilized to investigate the interannual variability of source, pathway, and dust loading associated with these dust outbreaks in East Asia. The monthly av-eraged aerosol optical thickness during the springtime from SeaWiFS will also be compared with the MODIS Deep Blue products.

Satellite Monitoring of Asian Dust Storms from SeaWiFS and MODIS: Source, pathway and Interannual Variability

NASA Technical Reports Server (NTRS)

Hsu, N. Christina

2007-01-01

Among the many components that contribute to air pollution, airborne mineral dust plays an important role due to its biogeochemical impact on the ecosystem and its radiative-forcing effect on the climate system. In East Asia, dust storms frequently accompany the cold and dry air masses that occur as part of springtime cold front systems. China's capital, Beijing, and other large cities are on the primary pathway of these dust storm plumes, and their passage over such population centers causes flight delays, pushes grit through windows and doors, and forces people indoors. Furthermore, during the spring these anthropogenic and natural air pollutants, once generated over the source regions, can be transported out of the boundary layer into the free troposphere and can travel thousands of kilometers across the Pacific into the United States and beyond. In this paper, we will demonstrate the capability of a new satellite algorithm to retrieve aerosol optical thickness and single scattering albedo over bright-reflecting surfaces such as urban areas and deserts. Such retrievals have been difficult to perform using previously available algorithms that use wavelengths from the mid-visible to the near IR because they have trouble separating the aerosol signal from the contribution due to the bright surface reflectance. The new algorithm, called Deep Blue, utilizes blue-wavelength measurements from instruments such as SeaWiFS and MODIS to infer the properties of aerosols, since the surface reflectance over land in the blue part of the spectrum is much lower than for longer wavelength channels. We have validated the satellite retrieved aerosol optical thickness with data from AERONET sunphotometers over desert and semi-desert regions. The comparisons show reasonable agreements between these two. These new satellite products will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from SeaWiFS and MODIS-like instruments. The multiyear satellite measurements since 1998 from SeaWiFS will be utilized to investigate the interannual variability of source, pathway, and dust loading associated with these dust outbreaks in East Asia. The monthly averaged aerosol optical thickness during the springtime from SeaWiFS will also be compared with the MODIS Deep Blue products.

Satellite Monitoring of Asian Dust Storms from SeaWiFS and MODIS: Source, Pathway, and Interannual Variability

NASA Technical Reports Server (NTRS)

Hsu, N. Christina; Tsay, S.-C.; Bettenhausen, C.; Salustro, C.; Jeong, M. J.

2010-01-01

Among the many components that contribute to air pollution, airborne mineral dust plays an important role due to its biogeochernical impact on the ecosystem and its radiative-forcing effect on the climate system. In East Asia, dust storms frequently accompany the cold and dry air masses that occur as part of springtime cold front systems. China's capital, Beijing, and other large cities are on the primary pathway of these dust storm plumes, and their passage over such population centers causes flight delays, pushes grit through windows and doors, and forces people indoors. Furthermore, during the spring these anthropogenic and natural air pollutants, once generated over the source regions, can be transported out of the boundary layer into the free troposphere and can travel thousands of kilometers across the Pacific into the United States and beyond. In this paper, we will demonstrate the capability of a new satellite algorithm to retrieve aerosol optical thickness and single scattering albedo over bright reflecting surfaces such as urban areas and deserts. Such retrievals have been difficult to perform using previously available algorithms that use wavelengths from the mid-visible to the near IR because they have trouble separating the aerosol signal from the contribution due to the bright surface reflectance. The new algorithm, called Deep Blue, utilizes blue-wavelength measurements from instruments such as SeaWiFS and MODIS to infer the properties of aerosols, since the surface reflectance over land in the blue part of the spectrum is much lower than for longer wavelength channels. We have validated the satellite retrieved aerosol optical thickness with data from AERONET sunphotometers over desert and semi-desert regions. The comparisons show reasonable agreements between these two. These new satellite products will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from SeaWiFS and MODIS-like instruments. The multiyear satellite measurements since 1998 from SeaWiFS will be utilized to investigate the interannual variability of source, pathway, and dust loading associated with these dust outbreaks in East Asia. The monthly averaged aerosol optical thickness during the springtime from SeaWiFS will also be compared with the MODIS Deep Blue products.

Satellite Monitoring of Asian Dust Storms from SeaWiFS and MODIS: Source, Pathway, and Interannual Variability

NASA Technical Reports Server (NTRS)

Hsu, N. Christina; Tsay, S.-C.; Bettenhausen, C.; Sayer, A.

2011-01-01

Among the many components that contribute to air pollution, airborne mineral dust plays an important role due to its biogeochemical impact on the ecosystem and its radiative-forcing effect on the climate system. In East Asia, dust storms frequently accompany the cold and dry air masses that occur as part of springtime cold front systems. China's capital, Beijing, and other large cities are on the primary pathway of these dust storm plumes, and their passage over such population centers causes flight delays, pushes grit through windows and doors, and forces peop Ie indoors. Furthermore, during the spring these anthropogenic and natural air pollutants, once generated over the source regions, can be tran sported out of the boundary layer into the free troposphere and can travel thousands of kilometers across the Pacific into the United States and beyond. In this paper, we will demonstrate the capability of a new satellite algorithm to retrieve aerosol optical thickness and single scattering albedo over brightreflecting surfaces such as urban areas and deserts. Such retrievals have been difficult to perform using previously available algorithms that use wavelengths from the mid-visible to the near IR because they have trouble separating the aerosol signal from the contribution due to the bright surface reflectance. The new algorithm, called Deep Blue, utilizes blue-wavelength measurements from instruments such as Sea WiFS and MODIS to infer the properties of aerosols, since the surface reflectance over land in the blue part of the spectrum is much lower than for longer wavelength channels. We have validated the satellite retrieved aerosol optical thickness with data from AERONET sunphotometers over desert and semi-desert regions. The comparisons show reasonable agreements between these two. These new satellite products will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from Sea WiFS and MODISlike instruments. The multiyear satellite measurements since 1998 from SeaWiFS will be utilized to investigate the interannual variability of source, pathway, and dust loading associated with these dust outbreaks in East Asia. The monthly averaged aerosol optical thickness during the springtime from SeaWiFS will also be compared with the MODIS Deep Blue products.

Far-ultraviolet imagery of the Orion Nebula

NASA Technical Reports Server (NTRS)

Carruthers, G. R.; Opal, C. B.

1977-01-01

Two electrographic cameras carried on a sounding rocket have yielded useful-resolution far-ultraviolet (1000-2000 A) imagery of the Orion Nebula. The brightness distribution in the images is consistent with a primary source which is due to scattering of starlight by dust grains, although an emission-line contribution, particularly in the fainter outer regions, is not ruled out. The results are consistent with an albedo of the dust grains that is high in the far-ultraviolet and which increases toward shorter wavelengths below 1230 A.

Trans-Pacific Transport of Saharan Dust to Western North America: A Case Study

NASA Technical Reports Server (NTRS)

Kendry, Ian G. M.; Strawbridge, Kevin B.; O'Neill, Norman; Macdonald, Anne Marie; Liu, Peter S. K.; Leaitch, W. Richard; Anlauf, Kurt G.; Jaegle, Lyatt; Fairlie, T. Duncan; Westphal, Douglas L.

2007-01-01

The first documented case of long range transport of Saharan dust over a pathway spanning Asia and the Pacific to Western North America is described. Crustal material generated by North African dust storms during the period 28 February - 3 March 2005 reached western Canada on 13-14 March 2005 and was observed by lidar and sunphotometer in the Vancouver region and by high altitude aerosol instrumentation at Whistler Peak. Global chemical models (GEOS-CHEM and NRL NAAPS) confirm the transport pathway and suggest source attribution was simplified in this case by the distinct, and somewhat unusual, lack of dust activity over Eurasia (Gobi and Takla Makan deserts) at this time. Over western North America, the dust layer, although subsiding close to the boundary layer, did not appear to contribute to boundary layer particulate matter concentrations. Furthermore, sunphotometer observations (and associated inversion products) suggest that the dust layer had only subtle optical impact (Aerosol Optical Thickness (Tau(sub a500)) and Angstrom exponent (Alpha(sub 440-870) were 0.1 and 1.2 respectively) and was dominated by fine particulate matter (modes in aerodynamic diameter at 0.3 and 2.5microns). High Altitude observations at Whistler BC, confirm the crustal origin of the layer (rich in Ca(++) ions) and the bi-modal size distribution. Although a weak event compared to the Asian Trans-Pacific dust events of 1998 and 2001, this novel case highlights the possibility that Saharan sources may contribute episodically to the aerosol burden in western North America.

77 FR 30953 - Approval and Promulgation of State Implementation Plans; State of Wyoming; Regional Haze Rule...

Federal Register 2010, 2011, 2012, 2013, 2014

2012-05-24

... the problem of visibility impairment in Class I areas, states need to develop strategies in... air corridors (CACs), mobile sources, and wind-blown dust, among other things. The EPA codified these...

77 FR 28825 - Approval, Disapproval and Promulgation of State Implementation Plans; State of Utah; Regional...

Federal Register 2010, 2011, 2012, 2013, 2014

2012-05-16

... transported over long distances, even hundreds of kilometers. Therefore, to effectively address the problem of... air corridors (CACs), mobile sources, and wind-blown dust, among other things. The EPA codified these...

77 FR 36043 - Approval and Promulgation of State Implementation Plans; New Mexico; Regional Haze Rule...

Federal Register 2010, 2011, 2012, 2013, 2014

2012-06-15

.... Therefore, to address effectively the problem of visibility impairment in Class I areas, states need to... development; and provisions to manage clean air corridors, mobile sources, and wind-blown dust, among other...

New Zealand as a Potential Source of Mineral Dust to the Atmosphere and Ocean during Glacial Periods

NASA Astrophysics Data System (ADS)

Koffman, B. G.; Goldstein, S. L.; Winckler, G.; Kaplan, M. R.; Bolge, L.; Cai, Y.; Recasens, C.; Koffman, T. N. B.

2017-12-01

The geochemical composition of sediments and dust can be used to trace their provenance, thereby providing insights into a range of Earth surface processes. During past glacial climates, much of the South Island of New Zealand (NZ) was blanketed by temperate erosive glacier systems, which significantly would have enhanced sediment production, including from associated active outwash plains. Such glacially-derived mineral dust from NZ may have impacted climate and ecological systems. In addition, dust and sediment can be used to trace downstream aeolian and oceanic transport. To this end, we systematically characterized the geochemical compositions of likely sediment- and dust-producing regions from the NZ South Island. We observe a strong relationship between sediment geochemical composition and geologic setting. Specifically, sediments from the central South Island, including the Canterbury Plains and Mackenzie Basin, where glaciers eroded mainly the Torlesse Greywacke, have a relatively homogenous isotopic composition, with 87Sr/86Sr = 0.7095-0.7165, ɛNd = -6.5 to -4.0, 206Pb/204Pb = 18.75-19.04, 207Pb/204Pb = 15.65-15.68, 208Pb/204Pb = 38.68-38.93. Southern South Island sediment sources, including southern Otago and Southland, show younger crust formation ages and more variable Sr and Nd isotopic compositions, reflecting the presence of Paleozoic volcanic complexes. Here 87Sr/86Sr = 0.7041-0.7140, ɛNd = -4.0 to +5.3, 206Pb/204Pb = 18.71-18.92, 207Pb/204Pb = 15.62-15.65, 208Pb/204Pb = 38.44-38.87. During the Last Glacial Maximum (LGM), glacial outwash and associated fluvial systems downstream were greatly expanded relative to present day, which could have provided regions for dust deflation - especially given a sea level lowering of 130 m. Due to processes linked to glaciations and lower sea levels, we suggest that the NZ South Island, though limited in extent compared to larger southern landmasses, may still have served as an important source of detritus during ice age climates.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Barbosa, C. L.; Blum, R. D.; Damineli, A.

In this paper we present the results of a mid-infrared study of G49.5-0.4, or W51A, part of the massive starbirth complex W51. Combining public data from the Spitzer IRAC camera, and Gemini mid-infrared camera T-ReCS at 7.73, 9.69, 12.33, and 24.56 μ m, with a spatial resolution of ∼0.″5, we have identified the mid-infrared counterparts of eight ultracompact H ii regions, showing that two radio sources are deeply embedded in molecular clouds and another is a cloud of ionized gas. From the T-ReCS data we have unveiled the central core of the W51 region, revealing massive young stellar candidates. Wemore » modeled the spectral energy distribution of the detected sources. The results suggest that the embedded objects are sources with spectral types ranging from B3 to O5, but the majority of the fits indicate stellar objects with B1 spectral types. We also present an extinction map of IRS 2, showing that a region with lower extinction corresponds to the region where a proposed jet of gas has impacted the foreground cloud. From this map, we also derived the total extinction toward the enigmatic source IRS 2E, which amounts to ∼60 mag in the V band. We calculated the color temperature due to thermal emission of the circumstellar dust of the detected sources; the temperatures are in the interval of ∼100–150 K, which corresponds to the emission of dust located at 0.1 pc from the central source. Finally, we show a possible mid-infrared counterpart of a detected source at millimeter wavelengths that was found by Zapata et al. to be a massive young stellar object undergoing a high accretion rate.« less

The importance of the diurnal cycle of Aerosol Optical Depth in West Africa

NASA Astrophysics Data System (ADS)

Kocha, Cécile; Tulet, Pierre; Lafore, Jean-Philippe; Flamant, Cyrille; Banks, Jamie; Marnas, Fabien; Brindley, Helen; Marsham, Jonh

2013-04-01

High resolution atmospheric simulations with the AROME model coupled with a dust module over West Africa for the whole of June 2006 and 2011 were used to calculate Aerosol Optical Depth (AOD). But the simulations showed a significant diurnal cycle of 0.2 in the dust AOD that could not be inferred from the MODIS Deep Blue satellite retrievals due to their time of overpass. The AROME AOD diurnal cycle have been compared to the new SEVIRI AOD retrievals in June 2011 and shows simlar AOD diurnal cycle. In fact, dust sources are mainly driven by the breakdown of the early morning low-level jet and by moist convection in the afternoon, leading to opposite diurnal cycles. The contribution in dust production is calculated for each processes. Moreover, simulations show that cloud cover significantly prevents the observation of AOD in convective areas. The under-sampling of the diurnal cycle by satellites like MODIS plus the impact of cloud masks on the space-borne AOD retrievals induce an underestimation of 0.28 (~40%) over the convective regions and an overestimation of 0.1 (17%) over morning source areas like Bodélé. Finally, the vertical dust distribution is explored via CALIPSO monthly mean from 2006 to 2011. The vertical dust distribution is a clue element to determine the dust raciative impact. Over the June month, the dust radiative impact affect the atmospheric energetic budget by an absorption of the short wave of 58W/m²/AOD into the atmosphere and a reduction of 50W/m²/AOD at the surface.

WMO SDS-WAS NAMEE Regional Center: Towards continuous evaluation of dust models in Northern Africa

NASA Astrophysics Data System (ADS)

Basart, Sara; García-Castillo, Gerardo; Cuevas, Emilio; Terradellas, Enric

2016-04-01

One of the most important activities of the Regional Center for Northern Africa, Middle East and Europe of the World Meteorological Organization's Sand and Dust Storm Warning Advisory and Assessment System (WMO SDS-WAS, http://sds-was.aemet.es) is the dust model intercomparison and forecast evaluation, which is deemed an indispensable service to the users and an invaluable tool to assess model skills. Currently, the Regional Center collects daily dust forecasts from models run by nine partners (BSC, ECMWF, NASA, NCEP, SEEVCCC, EMA, CNR-ISAC, NOA and UK Met Office). A multi-model ensemble has also been set up in an effort to provide added-value products to the users. The first problem to address the dust model evaluation is the scarcity of suitable routine observations near the Sahara, the world's largest source of mineral dust. The present contribution presents preliminary results of dust model evaluation using new observational datasets. The current routine evaluation of dust predictions is focused on total-column dust optical depth (DOD) and uses remote-sensing retrievals from sun-photometric (AERONET) and satellite (MODIS) measurements. However, most users of dust forecasts are interested in the concentration near the surface (in the air we breathe) rather than in the total column content. Therefore, evaluation of the predicted surface concentration is also necessary. In this context, the initiative of the African Monsoon Interdisciplinary Analysis (AMMA) International Program to establish permanent measuring stations in the Sahel is extremely important. Tapered Element Oscillating Microbalance (TEOM) monitors continuously record PM10 in M'Bour (Senegal); Cinzana (Mali) and Banizoumbou (Niger). This surface model evaluation is complemented with the PM10 observation from the Air Quality Control and Monitoring Network (AQCMN) of the Canary Islands (Spain). The region, located in the sub-tropical Eastern Atlantic (roughly 100 km west of the Moroccan coast), is frequently affected by intrusions of Saharan dust. Regional Node are evaluated during two years (2013-2014) with observations recorded in the Sahelian region and Canary Islands. Additionally, since the data sets of weather records have an excellent spatial and temporal coverage, observations of horizontal visibility included in meteorological reports are used as an alternative way to monitor dust events in near-real-time (NRT). Recently, a new visibility product that includes more than 1,500 METAR stations has implemented in the SDS-WAS NAMEE Regional Center. The present contribution also will demonstrate how the visibility can complement the information provided by other observing systems (air quality monitoring stations, sun photometers, vertical profilers or satellite products) and numerical simulations presenting its application in tracking several dust episodes. Otherwise, the vertical distribution of aerosol also influences the radiative effect at the top of the atmosphere, especially when aerosols have strong absorption of shortwave radiation. The free troposphere contribution to aerosol optical depth (AOD) and the altitude of lofted layers are provided thanks to the vertical profiling capability of the lidar/ceilomenter technique. Currently, a lidar located in Dakar (Senegal) and a ceilometer in Santa Cruz de Tenerife (Canary Islands, Spain) provide near-real-time (NRT) vertical profiles of aerosols, which are compared with those simulated by models.

PAHs underfoot: Contaminated dust from coal-tar sealcoated pavement is widespread in the United States

USGS Publications Warehouse

Van Metre, P.C.; Mahler, B.J.; Wilson, J.T.

2009-01-01

We reported in 2005 that runoff from parking lots treated with coal-tar-based sealcoat was a major source of polycyclic aromatic hydrocarbons (PAHs) to streams in Austin, Texas. Here we present new data from nine U. S. cities that show nationwide patterns in concentrations of PAHs associated with sealcoat Dust was swept from parking lots in six cities in the central and eastern U. S., where coal-tar-based sealcoat dominates use, and three cities in the western U. S., where asphalt-based sealcoat dominates use. For six central and eastern cities, median ?? PAH concentrations in dust from sealcoated and unsealcoated pavement are 2200 and 27 mg/kg, respectively. For three western cities, median ?? PAH concentrations in dust from sealcoated and unsealcoated pavement are similar and very low (2. 1 and 0. 8 mg/kg, respectively). Lakes in the central and eastern cities where pavement was sampled have bottom sediments with higher PAH concentrations than do those in the western cities relative to degree of urbanization. Bottom-sediment PAH assemblages are similar to those of sealcoated pavement dust regionally, implicating coal-tar-based sealcoat as a PAH source to the central and eastern lakes. Concentrations of benzo[a]pyrene in dust from coal-tar sealcoated pavement and adjacent soils greatly exceed generic soil screening levels, suggesting that research on human-health risk is warranted.

A new method for geochemical characterization of atmospheric mineral dust from polar ice cores: preliminary results from Talos Dome ice core (East Antarctica, Pacific-Ross Sea sector)

NASA Astrophysics Data System (ADS)

Baccolo, Giovanni; Delmonte, Barbara; Clemenza, Massimiliano; Previtali, Ezio; Maggi, Valter

2015-04-01

Assessing the elemental composition of atmospheric dust entrapped in polar ice cores is important for the identification of the potential dust sources and thus for the reconstruction of past atmospheric circulation, at local, regional and global scale. Accurate determination of major and trace elements in the insoluble fraction of dust extracted from ice cores is also useful to better understand some geochemical and biogeochemical mechanisms which are linked with the climate system. The extremely reduced concentration of dust in polar ice (typical Antarctic concentrations during interglacials are in the range of 10 ppb), the limited availability of such samples and the high risk of contamination make these analyses a challenge. A new method based on low background Instrumental Neutron Activation Analysis (INAA) was specifically developed for this kind of samples. The method allows the determination of the concentration of up to 35 elements in extremely reduced dust samples (20-30 μg). These elements span from major to trace and ultra-trace elements. Preliminary results from TALDICE (TALos Dome Ice CorE, East Antarctica, Pacific-Ross Sea Sector) ice core are presented along with results from potential source areas in Victoria Land. A set of 5 samples from Talos Dome, corresponding to the last termination, MIS3, MIS4 and MIS6 were prepared and analyzed by INAA.

Martian Dust Cycle

NASA Astrophysics Data System (ADS)

Cantor, B. A.; James, P. B.

The Mars Observer Camera (MOC), aboard Mars Global Surveyor (MGS), has completed approximately 3 consecutive Martian years of global monitoring, since entering its mapping orbit on March 9, 1999. MOC observations have shown the important role that dust devils and dust storms play in the Martian dust cycle on time scales ranging from semi-diurnally to interannually. These dust events have been observed across much of the planet from the depths of Hellas basin to the summit of Arsia Mons and range in size from10s of meters across (dust devils) to planet encircling (global dust veils). Though dust devils occur throughout most of the Martian year, each hemisphere has a "dust devil season" that generally follows the subsolar latitude and appears to be repeatable from year-to-year. An exception is NW Amazonis, which has frequent, large dust devils throughout northern spring and summer. MOC observations show no evidence that dust devils cause or lead to dust storms, however, observations do suggest that dust storms can initiate dust devil activity. Dust devils also might play a role in maintaining the low background dust opacity of the Martian atmosphere. Dust storms occur almost daily with few exceptions, with 1000s occurring each year in the present Martian environment, dispelling the notion of a "Classical Dust Storm Season". However, there does appear to be an annual dust storm cycle, with storms developing in specific locations during certain seasons and that some individual storm events are repeatable from year-to-year. The majority of storms develop near the receding seasonal polar cap edge or along the corresponding polar hood boundaries in their respective hemispheres, but they also occur in the northern plains, the windward side of the large shield volcanoes, and in low laying regions such as Hellas, Argyre, and Chryse. The rarest of dust events are the "Great Storms" or "Global Events", of which only 6 (4 "planet encircling" and 2 "global") have been observed to date. With MOC we have observed that global dust events are not individual storms but are composed of a number of local and regional storms (sources) and that they do not signify climatic changes, but are only short-term perturbations to the general interannually repeatable Martian dust storm cycle.

On the properties of dust and gas in the environs of V838 Monocerotis

NASA Astrophysics Data System (ADS)

Exter, K. M.; Cox, N. L. J.; Swinyard, B. M.; Matsuura, M.; Mayer, A.; De Beck, E.; Decin, L.

2016-12-01

Aims: We aim to probe the close and distant circumstellar environments of the stellar outburst object V838 Mon. Methods: Herschel far-infrared imaging and spectroscopy were taken at several epochs to probe the central point source and the extended environment of V838 Mon. PACS and SPIRE maps were used to obtain photometry of the dust immediately around V838 Mon, and in the surrounding infrared-bright region. These maps were fitted in 1d and 2d to measure the temperature, mass, and β of the two dust sources. PACS and SPIRE spectra were used to detect emission lines from the extended atmosphere of the star, which were then modelled to study the physical conditions in the emitting material. HIFI spectra were taken to measure the kinematics of the extended atmosphere but unfortunately yielded no detections. Results: Fitting of the far-infrared imaging of V838 Mon reveals 0.5-0.6 M⊙ of ≈19 K dust in the environs (≈2.7 pc) surrounding V838 Mon. The surface-integrated infrared flux (signifying the thermal light echo), and derived dust properties do not vary significantly between the different epochs. We measured the photometry of the point source. As the peak of the SED (Spectral Energy Distribution) lies outside the Herschel spectral range, it is only by incorporating data from other observatories and previous epochs that we can usefully fit the SED; with this we explicitly assume no evolution of the point source between the epochs. We find that warm dust with a temperature 300 K distributed over a radius of 150-200 AU. We fit the far-infrared lines of CO arising from the point source, from an extended environment around V838 Mon. Assuming a model of a spherical shell for this gas, we find that the CO appears to arise from two temperature zones: a cold zone (Tkin ≈ 18 K) that could be associated with the ISM or possibly with a cold layer in the outermost part of the shell, and a warm (Tkin ≈ 400 K) zone that is associated with the extended environment of V838 Mon within a region of radius of ≈210 AU. The SiO lines arise from a warm/hot zone. We did not fit the lines of H2O as they are far more dependent on the model assumed. Herschel is an ESA space observatory with science instruments provided by European-led Principal Investigator consortia and with important participation from NASA.

The LCO/Gemini-South campaign for Deep Impact target Comet 9P/Tempel 1: Temporally resolved wide-field narrowband imaging results

NASA Astrophysics Data System (ADS)

Lederer, S. M.; Osip, D. J.; Thomas-Osip, J. E.; DeBuizer, J. M.; Mondragon, L. A.; Schweiger, D. L.; Viehweg, J.; SB Collaboration

2005-08-01

An extensive observing campaign to monitor Comet 9P/Tempel 1 will be conducted from 20 June to 19 July, 2005 at Las Campanas Observatory, Chile. These observations will precede and follow the impact of the Deep Impact projectile, which is likely to create a crater on the nucleus that will act as a fresh active area on the surface of the comet. Discreet nucleus active areas, believed to be the source of coma gas and dust jets, will likely result in changing morphology in the coma. We present the initial results of the wide-field narrowband visible imaging of the comet. Data will be taken with the 2.5m DuPont telescope from 27 June - 9 July, following the comet from 4 rotations prior to impact, to 4 rotations after impact using the narrowband Hale-Bopp filters, including CN, C2, and two continuum filters. These data will allow an accurate determination of the rotation state of the embedded nucleus immediately preceding the impact event as well as a measure of any changes to the rotation state due to the impact. In addition, modeling of these data will provide the total dust and gas production rates from the unaltered nucleus compared to the enhanced dust and gas emission from the newly created active region and freely sublimating pieces of mantle material ejected into the coma by the impactor. We will monitor temporal changes (on hours and days time-scales) in the morphology of both the gas and refractory components. We will use coma morphology studies to estimate the dust and gas outflow velocities and infer the presence of discreet nucleus source regions (pre- and post-impact). Of particular interest is the study of the gas-to-dust ratio and the ratio of the minor carbon species emitted from the newly created active region relative to the pre-impact coma environment.

Snow Impurities on Central Asian Glaciers: Mineral Dust, Organic & Elemental Carbon

NASA Astrophysics Data System (ADS)

Schmale, J.; Kang, S.; Peltier, R.; Sprenger, M.; Guo, J.; Li, Y.; Zhang, Q.

2014-12-01

In Central Asia, 90 % of the population depend on water stored in glaciers and mountain snow cover. Accelerated melting can be induced by the deposition of e.g., mineral dust and black carbon that reduce the surface albedo. Data on source regions and chemical characteristics of snow impurities are however scarce in Central Asia. We studied aerosol deposited between summers of 2012 and 2013on three different glaciers in the Kyrgyz Republic. Samples were taken from two snow pits on the glacier Abramov in the northern Pamir and from one snow pit on Ak-Shiirak and Suek in the central Tien Shan. The snow was analyzed for elemental and total organic carbon, major ions and mineral dust. In addition, dissolved organic carbon was speciated by using the Aerodyne high-resolution time-of-flight aerosol spectrometer. Elevated mineral dust concentrations were found on all glaciers during summer and winter with lower annual average concentrations (20 mg l-1)in the northern Pamir (factor 5 to 6). Correlations between dust tracers varied, indicating different source regions. Average EC concentrations showed seasonal variation in the northern Pamir (> 100 μg l-1 in summer, < 30 μg l-1 in winter) while there was little variation throughout the year in the central Tien Shan (~ 200 μg l-1). Similarly, OC:EC ratios showed no seasonal cycle in that region averaging around 3. On Abramov, the ratio was significantly higher in winter (> 12) than in summer (< 4). The average O:C ratios across all glaciers ranged between 0.65 and 1.09, indicating a high degree of oxygenation which suggests long-range transport of the organic snow impurities. Marker substances such as potassium and mercury and their correlations suggest contribution from biomass burning emissions. Atmospheric measurements in August 2013 were conducted to obtain information on background aerosol characteristics in the remote high mountain areas. The average black carbon concentration was 0.26 μg/m³ (± 0.24 μg/m³).

Stable carbon and nitrogen isotopic compositions of ambient aerosols collected from Okinawa Island in the western North Pacific Rim, an outflow region of Asian dusts and pollutants

NASA Astrophysics Data System (ADS)

Kunwar, Bhagawati; Kawamura, Kimitaka; Zhu, Chunmao

2016-04-01

Stable carbon (δ13C) and nitrogen (δ15N) isotope ratios were measured for total carbon (TC) and nitrogen (TN), respectively, in aerosol (TSP) samples collected at Cape Hedo, Okinawa, an outflow region of Asian pollutants, during 2009-2010. The averaged δ13C and δ15N ratios are -22.2‰ and +12.5‰, respectively. The δ13C values are similar in both spring (-22.5‰) and winter (-22.5‰), suggesting the similar sources and/or source regions. We found that δ13C from Okinawa aerosols are ca. 2‰ higher than those reported from Chinese megacities probably due to photochemical aging of organic aerosols. A strong correlation (r = 0.81) was found between nss-Ca and TSP, suggesting that springtime aerosols are influenced from Asian dusts. However, carbonates in the Asian dusts were titrated with acidic species such as sulfuric acid and oxalic acid during atmospheric transport although two samples suggested the presence of remaining carbonate. No correlations were found between δ13C and tracer compounds (levoglucosan, elemental carbon, oxalic acid, and Na+). During winter and spring, coal burning is significant source in China. Based on isotopic mass balance, contribution of coal burning origin particles to total aerosol carbon was estimated as ca. 97% in winter, which is probably associated with the high emissions in China. Contribution of NO3- to TN was on average 45% whereas that of NH4+ was 18%. These results suggest that vehicular exhaust is an important source of TN in Okinawa aerosols. Concentration of water-soluble organic nitrogen (WSON) is higher in summer, suggesting that WSON is more emitted from the ocean in warmer season whereas inorganic nitrogen is more emitted in winter and spring from pollution sources in the Asian continent.

Aerosol Sources, Absorption, and Intercontinental Transport: Synergies among Models, Remote Sensing, and Atmospheric Measurements

NASA Technical Reports Server (NTRS)

Chin, Mian; Ginoux, Paul; Dubovik, Oleg; Holben, Brent; Kaufman, Yoram; chu, Allen; Anderson, Tad; Quinn, Patricia

2003-01-01

Aerosol climate forcing is one of the largest uncertainties in assessing the anthropogenic impact on the global climate system. This uncertainty arises from the poorly quantified aerosol sources, especially black carbon emissions, our limited knowledge of aerosol mixing state and optical properties, and the consequences of intercontinental transport of aerosols and their precursors. Here we use a global model GOCART to simulate atmospheric aerosols, including sulfate, black carbon, organic carbon, dust, and sea salt, from anthropogenic, biomass burning, and natural sources. We compare the model calculated aerosol extinction and absorption with those quantities from the ground-based sun photometer measurements from AERONET at several different wavelengths and the field observations from ACE-Asia, and model calculated total aerosol optical depth and fine mode fractions with the MODIS satellite retrieval. We will also estimate the intercontinental transport of pollution and dust aerosols from their source regions to other areas in different seasons.

Aerosol Sources, Absorption, and Intercontinental Transport: Synergies Among Models, Remote Sensing, and Atmospheric Measurements

NASA Technical Reports Server (NTRS)

Chin, Mian; Chu, Allen; Levy, Robert; Remer, Lorraine; Kaufman, Yoram; Dubovik, Oleg; Holben, Brent; Eck, Tom; Anderson, Tad; Quinn, Patricia

2004-01-01

Aerosol climate forcing is one of the largest uncertainties in assessing the anthropogenic impact on the global climate system. This uncertainty arises from the poorly quantified aerosol sources, especially black carbon emissions, our limited knowledge of aerosol mixing state and optical properties, and the consequences of intercontinental transport of aerosols and their precursors. Here we use a global model GOCART to simulate atmospheric aerosols, including sulfate, black carbon, organic carbon, dust, and sea salt, from anthropogenic, .biomass burning, and natural sources. We compare the model calculated aerosol extinction and absorption with those quantities from the ground-based sun photometer measurements from AERON" at several different wavelengths and the field observations from ACE-Asia, and model calculated total aerosol optical depth and fine mode fractions with the MODIS satellite retrieval. We will also estimate the intercontinental transport of pollution and dust aerosols from their source regions to other areas in different seasons.

Probing the infrared counterparts of diffuse far-ultraviolet sources in the Galaxy

NASA Astrophysics Data System (ADS)

Saikia, Gautam; Shalima, P.; Gogoi, Rupjyoti; Pathak, Amit

2017-12-01

Recent availability of high quality infrared (IR) data for diffuse regions in the Galaxy and external galaxies have added to our understanding of interstellar dust. A comparison of ultraviolet (UV) and IR observations may be used to estimate absorption, scattering and thermal emission from interstellar dust. In this paper, we report IR and UV observations for selective diffuse sources in the Galaxy. Using archival mid-infrared (MIR) and far-infrared (FIR) observations from Spitzer Space Telescope, we look for counterparts of diffuse far-ultraviolet (FUV) sources observed by the Voyager, Far Ultraviolet Spectroscopic Explorer (FUSE) and Galaxy Evolution Explorer (GALEX) telescopes in the Galaxy. IR emission features at 8 μm are generally attributed to Polycyclic Aromatic Hydrocarbon (PAH) molecules, while emission at 24 μm are attributed to Very Small Grains (VSGs). The data presented here is unique and our study tries to establish a relation between various dust populations. By studying the FUV-IR correlations separately at low and high latitude locations, we have identified the grain component responsible for the diffuse FUV emission.

New Insights into the Nature of Transition Disks from a Complete Disk Survey of the Lupus Star-forming Region

NASA Astrophysics Data System (ADS)

van der Marel, Nienke; Williams, Jonathan P.; Ansdell, M.; Manara, Carlo F.; Miotello, Anna; Tazzari, Marco; Testi, Leonardo; Hogerheijde, Michiel; Bruderer, Simon; van Terwisga, Sierk E.; van Dishoeck, Ewine F.

2018-02-01

Transition disks with large dust cavities around young stars are promising targets for studying planet formation. Previous studies have revealed the presence of gas cavities inside the dust cavities, hinting at recently formed, giant planets. However, many of these studies are biased toward the brightest disks in the nearby star-forming regions, and it is not possible to derive reliable statistics that can be compared with exoplanet populations. We present the analysis of 11 transition disks with large cavities (≥20 au radius) from a complete disk survey of the Lupus star-forming region, using ALMA Band 7 observations at 0.″3 (22–30 au radius) resolution of the 345 GHz continuum, 13CO and C18O 3–2 observations, and the spectral energy distribution of each source. Gas and dust surface density profiles are derived using the physical–chemical modeling code DALI. This is the first study of transition disks of large cavities within a complete disk survey within a star-forming region. The dust cavity sizes range from 20 to 90 au radius, and in three cases, a gas cavity is resolved as well. The deep drops in gas density and large dust cavity sizes are consistent with clearing by giant planets. The fraction of transition disks with large cavities in Lupus is ≳ 11 % , which is inconsistent with exoplanet population studies of giant planets at wide orbits. Furthermore, we present a hypothesis of an evolutionary path for large massive disks evolving into transition disks with large cavities.

The role of dust storms in total atmospheric particle concentrations at two sites in the western U.S.

USGS Publications Warehouse

Neff, Jason C.; Reynolds, Richard L.; Munson, Seth M.; Fernandez, Daniel; Belnap, Jayne

2013-01-01

Mineral aerosols are produced during the erosion of soils by wind and are a common source of particles (dust) in arid and semiarid regions. The size of these particles varies widely from less than 2 µm to larger particles that can exceed 50 µm in diameter. In this study, we present two continuous records of total suspended particle (TSP) concentrations at sites in Mesa Verde and Canyonlands National Parks in Colorado and Utah, USA, respectively, and compare those values to measurements of fine and coarse particle concentrations made from nearby samplers. Average annual concentrations of TSP at Mesa Verde were 90 µg m−3 in 2011 and at Canyonlands were 171 µg m−3 in 2009, 113 µg m−3 in 2010, and 134 µg m−3 in 2011. In comparison, annual concentrations of fine (diameter of 2.5 µm and below) and coarse (2.5–10 µm diameter) particles at these sites were below 10 µg m−3 in all years. The high concentrations of TSP appear to be the result of regional dust storms with elevated concentrations of particles greater than 10 µm in diameter. These conditions regularly occur from spring through fall with 2 week mean TSP periodically in excess of 200 µg m−3. Measurement of particles on filters indicates that the median particle size varies between approximately 10 µm in winter and 40 µm during the spring. These persistently elevated concentrations of large particles indicate that regional dust emission as dust storms and events are important determinants of air quality in this region.

Dust in the western U.S.: how biological, physical and human activities at the local scale interact to affect hydrologic function at the landscape scale (Invited)

NASA Astrophysics Data System (ADS)

Belnap, J.; Reheis, M. C.; Munson, S. M.

2009-12-01

Dryland regions constitute over 35% of terrestrial lands around the globe. Limited rainfall in these regions restricts plant growth and the spaces between vascular plants are often large. Most interspace soils are protected from wind erosion by the cover of rocks, physical crusts, and biological crusts (cyanobacteria, lichens, and mosses). However, disturbance of the soil surface in dryland regions (e.g., recreation, livestock, mining and energy exploration, military exercises, fire) reduces or eliminates the protective cover of the soils. Rising temperatures will reduce soil moisture and thus plant cover. Wind tunnel data show that most desert surfaces produce little sediment under typical wind speeds. However, disturbing the soil surface with vehicles, humans, or animals resulted in much higher sediment production from all surfaces tested, regardless of parent material, texture, or age of the soil surface. Synergist effects, such as surface disturbance occurring during drought periods in annualized plant communities, can create very large dust events. As surface disturbance, invasion, and drought are expected to increase in the future, an increase in dust production can be expected as well. Increased particulates in the air threaten human well-being through disease, highway accidents, and economic losses. Where dust losses are greater than the inputs, the source areas lose carbon and nutrients. These compounds are transferred to high elevation regions, where such fertilization likely impacts ecosystem function. Deposition of dust on the snowpack darkens the surface, increasing snowmelt by 30 days or more and exposing soils to evaporation, all of which decrease the quantity and quality of water in major streams and rivers. As increases occur in temperature, pumping of shallow aquifers, human activities, and invasion of exotic annual plants in dryland regions, the frequency, severity, and negative impact of dust storms is expected to increase as well. The implications of these future changes will be discussed.

Influence of Saharan dust outbreaks and carbon content on oxidative potential of water-soluble fractions of PM2.5 and PM10

NASA Astrophysics Data System (ADS)

Chirizzi, Daniela; Cesari, Daniela; Guascito, Maria Rachele; Dinoi, Adelaide; Giotta, Livia; Donateo, Antonio; Contini, Daniele

2017-08-01

Exposure to atmospheric particulate matter (PM) leads to adverse health effects although the exact mechanisms of toxicity are still poorly understood. Several studies suggested that a large number of PM health effects could be due to the oxidative potential (OP) of ambient particles leading to high concentrations of reactive oxygen species (ROS). The contribution to OP of specific anthropogenic sources like road traffic, biomass burning, and industrial emissions has been investigated in several sites. However, information about the OP of natural sources are scarce and no data is available regarding the OP during Saharan dust outbreaks (SDO) in Mediterranean regions. This work uses the a-cellular DTT (dithiothreitol) assay to evaluate OP of the water-soluble fraction of PM2.5 and PM10 collected at an urban background site in Southern Italy. OP values in three groups of samples were compared: standard characterised by concentrations similar to the yearly averages; high carbon samples associated to combustion sources (mainly road traffic and biomass burning) and SDO events. DTT activity normalised by sampled air volume (DTTV), representative of personal exposure, and normalised by collected aerosol mass (DTTM), representing source-specific characteristics, were investigated. The DTTV is larger for high PM concentrations. DTTV is well correlated with secondary organic carbon concentration. An increased DTTV response was found for PM2.5 compared to the coarse fraction PM2.5-10. DTTV is larger for high carbon content samples but during SDO events is statistically comparable with that of standard samples. DTTM is larger for PM2.5 compared to PM10 and the relative difference between the two size fractions is maximised during SDO events. This indicates that Saharan dust advection is a natural source of particles having a lower specific OP with respect to the other sources acting on the area (for water-soluble fraction). OP should be taken into account in epidemiological studies to evaluate the potential health risks associated to ROS in regions affected by high pollution events due to Saharan dust advection.

Advanced source apportionment of size-resolved trace elements at multiple sites in London during winter

DOE PAGES

Visser, S.; Slowik, Jay G.; Furger, M.; ...

2015-10-12

Here, trace element measurements in PM 10–2.5, PM 2.5–1.0 and PM 1.0–0.3 aerosol were performed with 2 h time resolution at kerbside, urban background and rural sites during the ClearfLo winter 2012 campaign in London. The environment-dependent variability of emissions was characterized using the Multilinear Engine implementation of the positive matrix factorization model, conducted on data sets comprising all three sites but segregated by size. Combining the sites enabled separation of sources with high temporal covariance but significant spatial variability. Separation of sizes improved source resolution by preventing sources occurring in only a single size fraction from having too smallmore » a contribution for the model to resolve. Anchor profiles were retrieved internally by analysing data subsets, and these profiles were used in the analyses of the complete data sets of all sites for enhanced source apportionment. A total of nine different factors were resolved (notable elements in brackets): in PM 10–2.5, brake wear (Cu, Zr, Sb, Ba), other traffic-related (Fe), resuspended dust (Si, Ca), sea/road salt (Cl), aged sea salt (Na, Mg) and industrial (Cr, Ni); in PM 2.5–1.0, brake wear, other traffic-related, resuspended dust, sea/road salt, aged sea salt and S-rich (S); and in PM 1.0–0.3, traffic-related (Fe, Cu, Zr, Sb, Ba), resuspended dust, sea/road salt, aged sea salt, reacted Cl (Cl), S-rich and solid fuel (K, Pb). Human activities enhance the kerb-to-rural concentration gradients of coarse aged sea salt, typically considered to have a natural source, by 1.7–2.2. These site-dependent concentration differences reflect the effect of local resuspension processes in London. The anthropogenically influenced factors traffic (brake wear and other traffic-related processes), dust and sea/road salt provide further kerb-to-rural concentration enhancements by direct source emissions by a factor of 3.5–12.7. The traffic and dust factors are mainly emitted in PM 10–2.5 and show strong diurnal variations with concentrations up to 4 times higher during rush hour than during night-time. Regionally influenced S-rich and solid fuel factors, occurring primarily in PM 1.0–0.3, have negligible resuspension influences, and concentrations are similar throughout the day and across the regions.« less

Advanced source apportionment of size-resolved trace elements at multiple sites in London during winter

DOE Office of Scientific and Technical Information (OSTI.GOV)

Visser, S.; Slowik, Jay G.; Furger, M.

Here, trace element measurements in PM 10–2.5, PM 2.5–1.0 and PM 1.0–0.3 aerosol were performed with 2 h time resolution at kerbside, urban background and rural sites during the ClearfLo winter 2012 campaign in London. The environment-dependent variability of emissions was characterized using the Multilinear Engine implementation of the positive matrix factorization model, conducted on data sets comprising all three sites but segregated by size. Combining the sites enabled separation of sources with high temporal covariance but significant spatial variability. Separation of sizes improved source resolution by preventing sources occurring in only a single size fraction from having too smallmore » a contribution for the model to resolve. Anchor profiles were retrieved internally by analysing data subsets, and these profiles were used in the analyses of the complete data sets of all sites for enhanced source apportionment. A total of nine different factors were resolved (notable elements in brackets): in PM 10–2.5, brake wear (Cu, Zr, Sb, Ba), other traffic-related (Fe), resuspended dust (Si, Ca), sea/road salt (Cl), aged sea salt (Na, Mg) and industrial (Cr, Ni); in PM 2.5–1.0, brake wear, other traffic-related, resuspended dust, sea/road salt, aged sea salt and S-rich (S); and in PM 1.0–0.3, traffic-related (Fe, Cu, Zr, Sb, Ba), resuspended dust, sea/road salt, aged sea salt, reacted Cl (Cl), S-rich and solid fuel (K, Pb). Human activities enhance the kerb-to-rural concentration gradients of coarse aged sea salt, typically considered to have a natural source, by 1.7–2.2. These site-dependent concentration differences reflect the effect of local resuspension processes in London. The anthropogenically influenced factors traffic (brake wear and other traffic-related processes), dust and sea/road salt provide further kerb-to-rural concentration enhancements by direct source emissions by a factor of 3.5–12.7. The traffic and dust factors are mainly emitted in PM 10–2.5 and show strong diurnal variations with concentrations up to 4 times higher during rush hour than during night-time. Regionally influenced S-rich and solid fuel factors, occurring primarily in PM 1.0–0.3, have negligible resuspension influences, and concentrations are similar throughout the day and across the regions.« less

Exploring the Longwave Radiative Effects of Dust Aerosols

NASA Technical Reports Server (NTRS)

Hansell, Richard A., Jr.

2012-01-01

Dust aerosols not only affect air quality and visibility where they pose a significant health and safety risk, but they can also play a role in modulating the energy balance of the Earth-atmosphere system by directly interacting with local radiative fields. Consequently, dust aerosols can impact regional climate patterns such as changes in precipitation and the evolution of the hydrological cycle. Assessing the direct effect of dust aerosols at the solar wavelengths is fairly straightforward due in part to the relatively large signal-to-noise ratio in broadband irradiance measurements. The longwave (LW) impacts, on the other hand, are rather difficult to ascertain since the measured dust signal level (10 Wm-2) is on the same order as the instrumental uncertainties. Moreover, compared to the shortwave (SW), limited experimental data on the LW optical properties of dust makes it a difficult challenge for constraining the LW impacts. Owing to the strong absorption features found in many terrestrial minerals (e.g., silicates and clays), the LW effects, although much smaller in magnitude compared to the SW, can still have a sizeable impact on the energetics of the Earth-atmosphere system, which can potentially trigger changes in the heat and moisture surface budgets, and dynamics of the atmosphere. The current endeavor is an integral part of an on-going research study to perform detailed assessments of dust direct aerosol radiative effects (DARE) using comprehensive global datasets from NASA Goddards mobile ground-based facility (cf. http://smartlabs.gsfc.nasa.gov/) during previous field experiments near key dust source regions. Here we examine and compare the results from two of these studies: the 2006 NASA African Monsoon Multidisciplinary Activities and the 2008 Asian Monsoon Years. The former study focused on transported Saharan dust at Sal Island (16.73N, 22.93W), Cape Verde along the west coast of Africa while the latter focused on Asian dust at Zhangye China (39.082N, 100.276E), a semi-arid region between the Taklimakan and Gobi deserts. NASA Goddards Giovanni system is used to help map out the spatial distribution of retrieved aerosol optical depths across the latter desert regions. 1-D radiative transfer model constrained by local measurements, including spectral photometry/interferometry and lidar for characterizing the spatiotemporal variability in dust properties and atmospheric conditions, is employed to evaluate the local instantaneous LW DARE of dust both at the surface and at the top of the atmosphere along with heating rate profiles for cloud-free atmospheres. The efficiency in LW DARE and its significance relative to the diurnally averaged SW effects are explored and compared in both studies. Found to be non-negligible, LW DARE is an important component in the study of regional climate variation with important implications for more detailed global assessments.

Infrared observations of OB star formation in NGC 6334

NASA Technical Reports Server (NTRS)

Harvey, P. M.; Gatley, I.

1982-01-01

Infrared photometry and maps from 2 to 100 microns are presented for three of the principal far infrared sources in NGC 6334. Each region is powered by two or more very young stars. The distribution of dust and ionized gas is probably strongly affected by the presence of the embedded stars; one of the sources is a blister H II region, another has a bipolar structure, and the third exhibits asymmetric temperature structure. The presence of protostellar objects throughout the region suggests that star formation has occurred nearly simultaneously in the whole molecular cloud rather than having been triggered sequentially from within.

Outflow and Infall in Star-forming Region L1221

NASA Astrophysics Data System (ADS)

Lee, Chin-Fei; Ho, Paul T. P.

2005-10-01

We have mapped the 3.3 mm continuum, CO, HCO+, N2H+, and CS emission around a nearby Class I source, IRAS 22266+6845, in the L1221 cometary dark cloud. L1221 is a complicated star-forming region. It hosts three infrared sources: a close binary consisting of an east source and a west source around the IRAS source position and a southeast source ~45" to the southeast (T. Bourke 2004, private communication). The east source is identified as the IRAS source. Continuum emission is seen around the east and southeast sources, probably tracing the dust around them. No continuum emission is seen toward the west source, probably indicating that there is not much dust there. An east-west molecular outflow is seen in CO, HCO+, and CS originated from around the binary. It is bipolar with an east lobe and a west lobe, both appearing as a wide-opening outflow shell originated from around the binary. It is likely powered by the east source, which shows a southeast extension along the outflow axis in the K' image. A ringlike envelope is seen in N2H+ around the binary surrounding the outflow waist. It is tilted with the major axis perpendicular to the outflow axis. The kinematics is well reproduced by a thin-disk model with both infall and rotation, and a column density peak in a ring. The ringlike envelope is not rotationally supported, as the rotation velocity is smaller than the infall velocity.

The regime of aerosol optical depth over Central Asia based on MODIS Aqua Deep Blue data

NASA Astrophysics Data System (ADS)

Floutsi, Athina; KorrasCarraca, Marios; Matsoukas, Christos; Biskos, George

2015-04-01

Atmospheric aerosols, both natural and anthropogenic, can affect the regional and global climate through their direct, indirect, and semi-direct effects on the radiative energy budget of the Earth-atmosphere system. To quantify these effects it is therefore important to determine the aerosol load, and an effective way to do that is by measuring the aerosol optical depth (AOD). In this study we investigate the spatial and temporal variability of the AOD over the climatically sensitive region of Central Asia (36° N - 50° N, 46° E - 75° E), which has significant sources of both natural and anthropogenic particles. The primary source of anthropogenic particles is fossil fuel combustion occurring mainly at oil refineries in the Caspian Sea basin. Natural particles originate mostly from the two deserts in the region (namely Kara-Kum and Kyzyl-Kum), where persistent dust activity is observed. Another source is the Aral Sea region, which due to its phenomenal desertification also drives an intense salt and dust transport from the exposed sea-bed to the surrounding regions. This transport is of particular interest because of health-hazardous materials contained in the Aral Sea sea-bed. For our analysis we use Level-3 daily MODIS - Aqua Dark Target - Deep Blue combined product, from the latest MODIS collection (006), available in 1° x 1° resolution (about 100 km x 100 km) over the period 2002-2014.Our first results indicate a significant spatial variability of the aerosol load over the study region. The data also show a clear seasonal cycle, with large aerosol load being associated with strong dust activity during spring and summer (AOD up to 0.5), and low during autumn and winter (AOD up to 0.4). In spring and summer significant aerosol load is observed in the Garabogazköl basin, Northeast and South-southeast Caspian Sea (offshore North Iran and Azerbaijan), as well as southwest of the Aral Sea. In the later region, the high AOD values can be explained by export of dust from the exposed sea-bed under strong northerly and north-easterly winds, and was found to be slightly larger during summer. From this analysis we have excluded the Aral Sea, over which the AOD values were extreme (up to 2.1 and 1.3 during July and January, respectively). The AOD exhibits statistically-significant increasing trend, with an ~40% mean regional relative change. The changes over are more pronounced over and around the Aral Sea, and are stronger during the warm period of the year (April to September). Our results suggest that these trends are associated with increased dust transport from the exposed Aral Sea sea-bed during the study period, which will be examined with the trends of the frequency and strength of aerosol events over central Asia, as well as their association with the Aral Sea desertification.

Boundary layer aerosol size distribution, mass concentration and mineralogical composition in Morocco and at Cape Verde Islands during SAMUM I-II

NASA Astrophysics Data System (ADS)

Kandler, K.; Lieke, K.

2009-04-01

The Saharan Mineral Dust Experiment (SAMUM) is dedicated to the understanding of the radiative effects of mineral dust. Two major field experiments were performed: A first joint field campaign took place at Ouarzazate and near Zagora, southern Morocco, from May 13 to June 7, 2006. Aircraft and ground based measurements of aerosol physical and chemical properties were carried out to collect a data set of surface and atmospheric columnar information within a major dust source. This data set combined with satellite data provides the base of the first thorough columnar radiative closure tests in Saharan dust. A second field experiment was conducted during January-February 2008, in the Cape Verde Islands region, where about 300 Tg of mineral dust are transported annually from Western Africa across the Atlantic towards the Caribbean Sea and the Amazon basin. Along its transport path, the mineral dust is expected to influence significantly the radiation budget - by direct and indirect effects - of the subtropical North Atlantic. We are lacking a radiative closure in the Saharan air plume. One focus of the investigation within the trade wind region is the spatial distribution of mixed dust/biomass/sea salt aerosol and their physical and chemical properties, especially with regard to radiative effects. We report on measurements of size distributions, mass concentrations and mineralogical composition conducted at the Zagora (Morocco) and Praia (Cape Verde islands) ground stations. The aerosol size distribution was measured from 20 nm to 500

The Martian Dust Devil Electron Avalanche: Laboratory Measurements of the E-Field Fortifying Effects of Dust-Electron Absorption

NASA Technical Reports Server (NTRS)

Farrell, W. M.; McLain, J. L.; Collier, M. R.; Keller, J. W.

2017-01-01

Analogous to terrestrial dust devils, charged dust in Mars dust devils should become vertically stratified in the convective features, creating large scale E-fields. This E-field in a Martian-like atmosphere has been shown to stimulate the development of a Townsend discharge (electron avalanche) that acts to dissipate charge in regions where charge build-up occurs. While the stratification of the charged dust is a source of the electrical energy, the uncharged particulates in the dust population may absorb a portion of these avalanching electrons, thereby inhibiting dissipation and leading to the development of anomalously large E-field values. We performed a laboratory study that does indeed show the presence of enhanced E-field strengths between an anode and cathode when dust-absorbing filaments (acting as particulates) are placed in the avalanching electron flow. Further, the E-field threshold condition to create an impulsive spark discharge increases to larger values as more filaments are placed between the anode and cathode. We conclude that the spatially separated charged dust creates the charge centers and E-fields in a dust devil, but the under-charged portion of the population acts to reduce Townsend electron dissipation currents, further fortifying the development of larger-than-expected E-fields.

Characteristics of mineral dust impacting the Persian Gulf

NASA Astrophysics Data System (ADS)

Ahmady-Birgani, Hesam; McQueen, Kenneth G.; Mirnejad, Hassan

2018-02-01

It is generally assumed that severe dust events in western Iran could be responsible for elevated levels of toxic and radioactive elements in the region. Over a period of 5 months, from January 2012 to May 2012, dust particles in the size range PM10 (i.e. <10 μm) were collected at Abadan, a site beside the Persian Gulf. The research aim was to compare chemical compositions of dust and aerosol samples collected during the non-dusty periods and during two severe dust events. Results of ICP-MS analysis of components indicate that during dust events the concentrations of major elements such as Ca, Mg, Al and K increase relative to ambient conditions when Fe and trace elements such as Cu, Cr, Ni, Pb and Zn are in higher proportions. Toxic trace elements that are generally ascribed to human activities, including industrial and urban pollution, are thus proportionately more abundant in the dust under calm conditions than during dust events, when their concentration is diluted by more abundant mineral particles of quartz, calcite and clay. The variability of chemical species during two dust events, noted by tracking the dust plumes in satellite images, was also assessed and the results relate to two different source areas, namely northern Iraq and northwestern Syria.

Interannual Variations in Aerosol Sources and Their Impact on Orographic Precipitation Over California's Central Sierra Nevada

NASA Technical Reports Server (NTRS)

Creamean, J. M.; Ault, A. P.; White, A. B.; Neiman, P. J.; Ralph, F. M.; Minnis, Patrick; Prather, K. A.

2014-01-01

Aerosols that serve as cloud condensation nuclei (CCN) and ice nuclei (IN) have the potential to profoundly influence precipitation processes. Furthermore, changes in orographic precipitation have broad implications for reservoir storage and flood risks. As part of the CalWater I field campaign (2009-2011), the impacts of aerosol sources on precipitation were investigated in the California Sierra Nevada. In 2009, the precipitation collected on the ground was influenced by both local biomass burning (up to 79% of the insoluble residues found in precipitation) and long-range transported dust and biological particles (up to 80% combined), while in 2010, by mostly local sources of biomass burning and pollution (30-79% combined), and in 2011 by mostly long-range transport from distant sources (up to 100% dust and biological). Although vast differences in the source of residues was observed from year-to-year, dust and biological residues were omnipresent (on average, 55% of the total residues combined) and were associated with storms consisting of deep convective cloud systems and larger quantities of precipitation initiated in the ice phase. Further, biological residues were dominant during storms with relatively warm cloud temperatures (up to -15 C), suggesting these particles were more efficient IN compared to mineral dust. On the other hand, lower percentages of residues from local biomass burning and pollution were observed (on average 31% and 9%, respectively), yet these residues potentially served as CCN at the base of shallow cloud systems when precipitation quantities were low. The direct connection of the source of aerosols within clouds and precipitation type and quantity can be used in models to better assess how local emissions versus long-range transported dust and biological aerosols play a role in impacting regional weather and climate, ultimately with the goal of more accurate predictive weather forecast models and water resource management.

Interannual Variations in Aerosol Sources and Their Impact on Orographic Precipitation over California's Central Sierra Nevada

NASA Astrophysics Data System (ADS)

Creamean, J.; Ault, A. P.; White, A. B.; Neiman, P. J.; Minnis, P.; Prather, K. A.

2014-12-01

Aerosols that serve as cloud condensation nuclei (CCN) and ice nuclei (IN) have the potential to profoundly influence precipitation processes. Furthermore, changes in orographic precipitation have broad implications for reservoir storage and flood risks. As part of the CalWater I field campaign (2009-2011), the impacts of aerosol sources on precipitation were investigated in the California Sierra Nevada Mountains. In 2009, the precipitation collected on the ground was influenced by both local biomass burning and long-range transported dust and biological particles, while in 2010, by mostly local sources of biomass burning and pollution, and in 2011 by mostly long-range transport of dust and biological particles from distant sources. Although vast differences in the sources of residues were observed from year-to-year, dust and biological residues were omnipresent (on average, 55% of the total residues combined) and were associated with storms consisting of deep convective cloud systems and larger quantities of precipitation initiated in the ice phase. Further, biological residues were dominant during storms with relatively warm cloud temperatures (up to -15°C), suggesting biological components were more efficient IN than mineral dust. On the other hand, when precipitation quantities were lower, local biomass burning and pollution residues were observed (on average 31% and 9%, respectively), suggesting these residues potentially served as CCN at the base of shallow cloud systems and that lower level polluted clouds of storm systems produced less precipitation than non-polluted (i.e., marine) clouds. The direct connection of the sources of aerosols within clouds and precipitation type and quantity can be used in models to better assess how local emissions versus long-range transported dust and biological aerosols play a role in impacting regional weather and climate, ultimately with the goal of more accurate predictive weather forecast models and water resource management.

Dust emission at Franklin Lake Playa, Mojave Desert (USA): Response to meteorological and hydrologic changes 2005-2008

USGS Publications Warehouse

Reynolds, Richard L.; Bogle, Rian; Vogel, John; Goldstein, Harland L.; Yount, James

2009-01-01

Playa type, size, and setting; playa hydrology; and surface-sediment characteristics are important controls on the type and amount of atmospheric dust emitted from playas. Soft, evaporite-rich sediment develops on the surfaces of some Mojave Desert (USA) playas (wet playas), where the water table is shallow (< 4 m). These areas are sources of atmospheric dust because of continuous or episodic replenishment of wind-erodible salts and disruption of the ground surface during salt formation by evaporation of ground water. Dust emission at Franklin Lake playa was monitored between March 2005 and April 2008. The dust record, based on day-time remote digital camera images captured during high wind, and compared with a nearby precipitation record, shows that aridity suppresses dust emission. High frequency of dust generation appears to be associated with relatively wet periods, identified as either heavy precipitation events or sustained regional precipitation over a few months. Several factors may act separately or in combination to account for this relation. Dust emission may respond rapidly to heavy precipitation when the dissolution of hard, wind-resistant evaporite mineral crusts is followed by the development of soft surfaces with thin, newly formed crusts that are vulnerable to wind erosion and (or) the production of loose aggregates of evaporite minerals that are quickly removed by even moderate winds. Dust loading may also increase when relatively high regional precipitation leads to decreasing depth to the water table, thereby increasing rates of vapor discharge, development of evaporite minerals, and temporary softening of playa surfaces. The seasonality of wind strength was not a major factor in dust-storm frequency at the playa. The lack of major dust emissions related to flood-derived sediment at Franklin Lake playa contrasts with some dry-lake systems elsewhere that may produce large amounts of dust from flood sediments. Flood sediments do not commonly accumulate on the surface of Franklin Lake playa because through-going drainage prevents frequent inundation and deposition of widespread flood sediment.

Physical characterization, magnetic measurements, REE geochemistry and biomonitoring of dust load accumulated during a protracted winter fog period and their implications.

PubMed

Chakarvorty, Munmun; Pati, Jayanta Kumar; Patil, Shiva Kumar; Shukla, Swati; Niyogi, Ambalika; Saraf, Arun Kumar

2014-05-01

The winter fog in India is a recurrent phenomenon for more than a decade now affecting the entire Himalayan and sub-Himalayan regions covering an area of nearly 500,000 km(2). Every winter (December-January), the air and surface transports in cities of northern India (Amritsar, New Delhi, Agra, Gwalior, Kanpur, Lucknow, and Allahabad) are severely disrupted with visibility reduced to <50 m at times. Since dust particles are known to act as nuclei for the fog formation, this study is aimed to carry out physicochemical characterization of the dust particulates accumulated during a protracted fog period from one of the severely fog affected cities of north India (Allahabad; 25°27'33.40″N-81°52'45.47″E). The dust-loaded tree leaves belonging to Ficus bengalensis and Ficus religiosa from 50 different locations between January 24 and 31, 2010 are sampled and characterized. The mass of dust, color, grain shape, size, phase constituents, and mineral magnetic parameters, such as magnetic susceptibility, SIRM, χ fd%, and S-ratio, show minor variation and the regional influence outweighs local anthropogenic contributions. The dust compositions show fractionated rare earth element pattern with a pronounced negative Eu anomaly similar to upper continental crust and further suggesting their derivation from sources located in parts of north and central India.

Testing an advanced satellite technique for dust detection as a decision support system for the air quality assessment

NASA Astrophysics Data System (ADS)

Falconieri, Alfredo; Filizzola, Carolina; Femiano, Rossella; Marchese, Francesco; Sannazzaro, Filomena; Pergola, Nicola; Tramutoli, Valerio; Di Muro, Ersilia; Divietri, Mariella; Crisci, Anna Maria; Lovallo, Michele; Mangiamele, Lucia; Vaccaro, Maria Pia; Palma, Achille

2014-05-01

In order to correctly apply the European directive for air quality (2008/50/CE), local Authorities are often requested to discriminate the possible origin (natural/anthropic) of anomalous concentration of pollutants in the air (art.20 Directive 2008/50/CE). In this framework, it's been focused on PM10 and PM2,5 concentrations and sources. In fact, depending on their origin, appropriate counter-measures can be taken devoted to prevent their production (e.g. by traffic restriction) or simply to reduce their impact on citizen health (e.g. information campaigns). In this context suitable satellite techniques can be used in order to identify natural sources (particularly Saharan dust, but also volcanic ash or forest fire smoke) that can be responsible of over-threshold concentration of PM10/2,5 in populated areas. In the framework of the NIBS (Networking and Internationalization of Basilicata Space Technologies) project, funded by the Basilicata Region within the ERDF 2007-2013 program, the School of Engineering of University of Basilicata, the Institute of Methodologies for Environmental Analysis of National Research Council (IMAA-CNR) and the Regional Agency for the Protection of the Environment of Basilicata Region (ARPAB) have started a collaboration devoted to assess the potential of the use of advanced satellite techniques for Saharan dust events identification to support ARPAB activities related to the application of the European directive for air quality (2008/50/CE) in Basilicata region. In such a joint activity, the Robust Satellite Technique (RST) approach has been assessed and tested as a decision support system for monitoring and evaluating air quality at local and regional level. In particular, RST-DUST products, derived by processing high temporal resolution data provided by SEVIRI (Spinning Enhanced Visible and Infrared Imager) sensor on board Meteosat Second Generation platforms, have been analysed together with PM10 measurements performed by the ground-based stations operated by ARPAB. Such an inter-comparison was devoted to investigate possible PM10 over-threshold occurrences and to better evaluate their possible causes (i.e. anthropogenic and/or natural sources). The analysis demonstrated the added value of an independent, automatic and unsupervised satellite based system (capable of discriminating over-threshold PM10 data produced by natural source from the ones occurred because of anthropogenic causes) in supporting the decisions of the considered end-user (ARPAB) in a pre-operational context.

Multi-Wavelength Study of W40 HII Region

NASA Astrophysics Data System (ADS)

Shenoy, Sachindev S.; Shuping, R.; Vacca, W. D.

2013-01-01

W40 is an HII region (Sh2-64) within the Serpens molecular cloud in the Aquila rift region. Recent near infrared spectroscopic observations of the brightest members of the central cluster of W40 reveal that the region is powered by at least three early B-type stars and one late O-type star. Near and mid-infrared spectroscopy and photometry, combined with SED modeling of these sources, suggest that the distance to the cluster is between 455 and 535 pc, with about 10 mag of visual extinction. Velocity and extinction measurement of all the nearby regions i.e. Serpens main, Aquila rift, and MWC297 suggest that the entire system (including the W40 extended emission) is associated with the extinction wall at 260 pc. Here we present some preliminary results of a multi-wavelength study of the central cluster and the extended emission of W40. We used Spitzer IRAC data to measure accurate photometry of all the point sources within 4.32 pc of W40 via PRF fitting. This will provide us with a complete census of YSOs in the W40 region. The Spitzer data are combined with publicly available data in 2MASS, WISE and Hershel archives and used to model YSOs in the region. The SEDs and near-IR colors of all the point sources should allow us to determine the age of the central cluster of W40. The results from this work will put W40 in a proper stellar evolutionary context. After subtracting the point sources from the IRAC images, we are able to study the extended emission free from point source contamination. We choose a few morphologically interesting regions in W40 and use the data to model the dust emission. The results from this effort will allow us to study the correlation between dust properties and the large scale physical properties of W40.

OT2_dardila_2: PACS Photometry of Transiting-Planet Systems with Warm Debris Disks

NASA Astrophysics Data System (ADS)

Ardila, D.

2011-09-01

Dust in debris disks is produced by colliding or evaporating planetesimals, the remnant of the planet formation process. Warm dust disks, known by their emission at =<24 mic, are rare (4% of FGK main-sequence stars), and specially interesting because they trace material in the region likely to host terrestrial planets, where the dust has very short dynamical lifetimes. Dust in this region comes from very recent asteroidal collisions, migrating Kuiper Belt planetesimals, or migrating dust. NASA's Kepler mission has just released a list of 1235 candidate transiting planets, and in parallel, the Wide-Field Infrared Survey Explorer (WISE) has just completed a sensitive all-sky mapping in the 3.4, 4.6, 12, and 22 micron bands. By cross-identifying the WISE sources with Kepler candidates as well as with other transiting planetary systems we have identified 21 transiting planet hosts with previously unknown warm debris disks. We propose Herschel/PACS 100 and 160 micron photometry of this sample, to determine whether the warm dust in these systems represents stochastic outbursts of local dust production, or simply the Wien side of emission from a cold outer dust belt. These data will allow us to put constraints in the dust temperature and infrared luminosity of these systems, allowing them to be understood in the context of other debris disks and disk evolution theory. This program represents a unique opportunity to exploit the synergy between three great space facilities: Herschel, Kepler, and WISE. The transiting planet sample hosts will remain among the most studied group of stars for the years to come, and our knowledge of their planetary architecture will remain incomplete if we do not understand the characteristics of their debris disks.

Environmental lead pollution threatens the children living in the Pearl River Delta region, China.

PubMed

Chen, Jianmin; Tong, Yongpeng; Xu, Jiazhang; Liu, Xiaoli; Li, Yulan; Tan, Mingguang; Li, Yan

2012-09-01

The objective of this study is to determine children's blood lead levels and identify sources of lead exposure. Childhood lead exposure constitutes a major pediatric health problem today in China. A blood lead screening survey program for children in the age group of 2-12 years residing in Pearl River Delta region, south of China, was carried out from Dec 2007 to Jan 2008. Blood lead levels and lead isotope ratios of a total of 761 participants were assessed by inductively coupled plasma mass spectroscopy. Measurements of urban environmental samples for source identification of children lead exposure were also performed. The geometric mean value of the children's blood lead levels was 57.05 μg/L, and 9.6% of them were higher than 100 μg/L. The blood lead levels were still much higher than those in developed countries. Based on the data of environmental lead source inventories, lead isotopic tracing revealed that there is about 6.7% past used gasoline Pb embedded in Shenzhen residential dust and about 15.6% in Guangzhou dust, respectively.

Effect of ecological restoration programs on dust concentrations in the North China Plain: a case study

NASA Astrophysics Data System (ADS)

Long, Xin; Tie, Xuexi; Li, Guohui; Cao, Junji; Feng, Tian; Zhao, Shuyu; Xing, Li; An, Zhisheng

2018-05-01

In recent decades, the Chinese government has made a great effort in initiating large-scale ecological restoration programs (ERPs) to reduce the dust concentrations in China, especially for dust storm episodes. Using the Moderate Resolution Imaging Spectroradiometer (MODIS) land cover product, the ERP-induced land cover changes are quantitatively evaluated in this study. Two obvious vegetation protective barriers arise throughout China from the southwest to the northeast, which are well known as the Green Great Wall (GGW). Both the grass GGW and forest GGW are located between the dust source region (DSR) and the densely populated North China Plain (NCP). To assess the effect of ERPs on dust concentrations, a regional transport/dust model (WRF-DUST, Weather Research and Forecast model with dust) is applied to investigate the evolution of dust plumes during a strong dust storm episode from 2 to 8 March 2016. The WRF-DUST model generally performs reasonably well in reproducing the temporal variations and spatial distributions of near-surface [PMC] (mass concentration of particulate matter with aerodynamic diameter between 2.5 and 10 µm) during the dust storm event. Sensitivity experiments have indicated that the ERP-induced GGWs help to reduce the dust concentration in the NCP, especially in BTH (Beijing, Tianjin, and Hebei). When the dust storm is transported from the upwind DSR to the downwind NCP, the [PMC] reduction ranges from -5 to -15 % in the NCP, with a maximum reduction of -12.4 % (-19.2 µg m-3) in BTH and -7.6 % (-10.1 µg m-3) in the NCP. We find the dust plumes move up to the upper atmosphere and are transported from the upwind DSR to the downwind NCP, accompanied by dust decrease. During the episode, the forest GGW is nonsignificant in dust concentration control because it is of benefit for dry deposition and not for emission. Conversely, the grass GGW is beneficial in controlling dust erosion and is the dominant reason for [PMC] decrease in the NCP. Because the air pollution is severe in eastern China, especially in the NCP, and the contribution of dust episodes is significant, the reduction of dust concentrations will have important effects on severe air pollution. This study illustrates the considerable contribution of ERPs to the control of air pollution in China, especially in springtime.

Source apportionment of fine particulate matter measured in an industrialized coastal urban area of South Texas

NASA Astrophysics Data System (ADS)

Karnae, Saritha; John, Kuruvilla

2011-07-01

Corpus Christi is a growing industrialized urban airshed in South Texas impacted by local emissions and regional transport of fine particulate matter (PM 2.5). Positive matrix factorization (PMF2) technique was used to evaluate particulate matter pollution in the urban airshed by estimating the types of sources and its corresponding mass contributions affecting the measured ambient PM 2.5 levels. Fine particulate matter concentrations by species measured during July 2003 through December 2008 at a PM 2.5 speciation site were used in this study. PMF2 identified eight source categories, of which secondary sulfates were the dominant source category accounting for 30.4% of the apportioned mass. The other sources identified included aged sea salt (18.5%), biomass burns (12.7%), crustal dust (10.1%), traffic (9.7%), fresh sea salt (8.1%), industrial sources (6%), and a co-mingled source of oil combustion & diesel emissions (4.6%). The apportioned PM mass showed distinct seasonal variability between source categories. The PM levels in Corpus Christi were affected by biomass burns in Mexico and Central America during April and May, sub-Saharan dust storms from Africa during the summer months, and a continental haze episode during August and September with significant transport from the highly industrialized areas of Texas and the neighboring states. Potential source contribution function (PSCF) analysis was performed and it identified source regions and the influence of long-range transport of fine particulate matter affecting this urban area.

A long Saharan dust event over the western Mediterranean: Lidar, Sun photometer observations, and regional dust modeling

NASA Astrophysics Data System (ADS)

PéRez, C.; Nickovic, S.; Baldasano, J. M.; Sicard, M.; Rocadenbosch, F.; Cachorro, V. E.

2006-08-01

A long Saharan dust event affected the western Mediterranean in the period 12-28 June 2002. Dust was present mainly between 1- and 5-km height affecting most parts of the Iberian Peninsula and reaching western/central Europe. Intensive backscatter lidar observations over Barcelona (Spain) and Sun photometer data from two stations (El Arenosillo, Spain, and Avignon, France) are used to evaluate different configurations the Dust Regional Atmospheric Modeling (DREAM) system. DREAM currently operates dust forecasts over the Mediterranean region (http://www.bsc.es/projects/earthscience/DREAM/) considering four particle size bins while only the first two are relevant for long-range transport analysis since their life time is larger than 12 hours. A more detailed bin method is implemented, and two different dust distributions at sources are compared to the operational version. Evaluations are performed at two wavelengths (532 and 1064 nm). The dust horizontal and vertical structure simulated by DREAM shows very good qualitative agreement when compared to SeaWIFS satellite images and lidar height-time displays over Barcelona. When evaluating the modeled aerosol optical depth (AOD) against Sun photometer data, significant improvements are achieved with the use of the new detailed bin method. In general, the model underpredicts the AOD for increasing Ångström exponents because of the influence of anthropogenic pollution in the boundary layer. In fact, the modeled AOD is highly anticorrelated with the observed Ångström exponents. Avignon shows higher influence of small anthropogenic aerosols which explains the better results of the model at the wavelength of 1064 nm over this location. The uncertainties of backscatter lidar inversions (20-30%) are in the same order of magnitude as the differences between the model experiments. Better model results are obtained when comparing to lidar because most of the anthropogenic effect is removed.

Dust and biological aerosols from the Sahara and Asia influence precipitation in the western U.S.

PubMed

Creamean, Jessie M; Suski, Kaitlyn J; Rosenfeld, Daniel; Cazorla, Alberto; DeMott, Paul J; Sullivan, Ryan C; White, Allen B; Ralph, F Martin; Minnis, Patrick; Comstock, Jennifer M; Tomlinson, Jason M; Prather, Kimberly A

2013-03-29

Winter storms in California's Sierra Nevada increase seasonal snowpack and provide critical water resources and hydropower for the state. Thus, the mechanisms influencing precipitation in this region have been the subject of research for decades. Previous studies suggest Asian dust enhances cloud ice and precipitation, whereas few studies consider biological aerosols as an important global source of ice nuclei (IN). Here, we show that dust and biological aerosols transported from as far as the Sahara were present in glaciated high-altitude clouds coincident with elevated IN concentrations and ice-induced precipitation. This study presents the first direct cloud and precipitation measurements showing that Saharan and Asian dust and biological aerosols probably serve as IN and play an important role in orographic precipitation processes over the western United States.

Application and verification of the NMMB/BSC-CTM forecast for solar energy

NASA Astrophysics Data System (ADS)

Soret, Albert; Serradell, Kim; Piot, Matthias; Ortega, Daniel; Obiso, Vincenzo; Jorba, Oriol

2016-04-01

In the beginning of April 2014, northern Europe was affected by a mineral dust intrusion. On 4 April 2014, the power prediction for German solar installations was estimated as 21 GW, whereas the measured power production merely reached 11 GW. This strong overestimation significantly affected the hourly price in the wholesale electricity market: prices were firstly assessed at around 27 € /MWh but rapidly reached a level close to 150 € /MWh after recognizing the lack of solar output. It has been found that a large proportion of the uncertainty of existing NWP models can be attributed to the lack of accurate aerosol data used in order to model solar radiation. Despite the advancements in the modelling of aerosol-cloud interactions, current meteorological models use parameterizations made mostly for climate considerations (generally monthly-based). In this contribution, we analyse model results of the direct radiative effect of mineral dust over Germany at the beginning of April 2014. For that, the NMMB/BSC Chemical Transport Model (NMMB/BSC-CTM) is applied on a regional domain at 0.1° horizontal resolution. The NMMB/BSC-CTM is a new on-line chemical weather prediction system coupling atmospheric and chemistry processes. In the radiation module of the model, mineral dust is treated as a radiatively active substance interacting both short and longwave radiation. The impact of the mineral dust outbreaks on meteorology is discussed by comparing model forecasts meteorological observations. The analysis focuses on the performance of the NMMB/BSC-CTM to simulate the radiative effects of a mineral dust intrusion far from source regions. Model results would help to illustrate the added value of on-line models for long term analysis of solar resource. On-going developments: integration of anthropogenic sources and implementation of indirect radiative effects will be also presented.

ALMA deep field in SSA22: Survey design and source catalog of a 20 arcmin2 survey at 1.1 mm

NASA Astrophysics Data System (ADS)

Umehata, Hideki; Hatsukade, Bunyo; Smail, Ian; Alexander, David M.; Ivison, Rob J.; Matsuda, Yuichi; Tamura, Yoichi; Kohno, Kotaro; Kato, Yuta; Hayatsu, Natsuki H.; Kubo, Mariko; Ikarashi, Soh

2018-06-01

To search for dust-obscured star-formation activity in the early Universe, it is essential to obtain a deep and wide submillimeter/millimeter map. The advent of the Atacama Large Millimeter/submillimeter Array (ALMA) has enabled us to obtain such maps with sufficiently high spatial resolution to be free from source confusion. We present a new 1.1 mm-wave map obtained by ALMA in the SSA22 field. The field contains a remarkable proto-cluster at z = 3.09; therefore, it is an ideal region to investigate the role of a large-scale cosmic web on dust-obscured star formation. The typical 1σ depth of our map is 73 μJy beam-1 with a {0^{^''.}5} resolution. Combining the present survey with earlier, archived observations, we map an area of 20 arcmin2 (71 comoving Mpc2 at z = 3.09). Within the combined survey area we have detected 35 sources at a signal-to-noise ratio (S/N) >5, with flux densities of S1.1mm = 0.43-5.6 mJy, equivalent to star-formation rates of ≳100-1000 M⊙ yr-1 at z = 3.09, for a Chabrier initial mass function: 17 sources out of 35 are new detections. The cumulative number counts show an excess by a factor of three to five compared to blank fields. The excess suggests enhanced, dust-enshrouded star-formation activity in the proto-cluster on a 10 comoving Mpc scale, indicating accelerated galaxy evolution in this overdense region.

Precipitation chemistry over urban, rural and high altitude Himalayan stations in eastern India

NASA Astrophysics Data System (ADS)

Roy, Arindam; Chatterjee, Abhijit; Tiwari, Suresh; Sarkar, Chirantan; Das, Sanat Kumar; Ghosh, Sanjay Kumar; Raha, Sibaji

2016-11-01

A study of precipitation (rainwater) chemistry during the two consecutive summer monsoon seasons of 2013 and 2014 at a high altitude station (2200 m asl) at eastern Himalaya region (Darjeeling); a typical metropolitan urban location (Kolkata), and a rural environment near the Bay of Bengal (Falta) was conducted. The volume-weighted mean (VWM) concentration shows that total ionic composition was maximum over Kolkata (391 μeq l- 1) followed by Falta (204 μeq l- 1) and Darjeeling (64 μeq l- 1). 85% rain samples were alkaline over Kolkata, whereas, 55 and 65% samples were acidic over Falta and Darjeeling respectively. Ca2 + was the most potential species to completely neutralize the acidity over Kolkata, whereas, NH4+ was the potential species to partially neutralize the acidity over Falta and Darjeeling. The deposition fluxes of anthropogenic and dust species over Kolkata was remarkably higher than Falta and Darjeeling. Anthropogenic and dust chemical species in rainwater were found to be dominant over Kolkata and Falta when the air masses passes from the polluted continental region. Rainwater acidity over Darjeeling was highest when air masses arrived from the Arabian Sea compared to air masses from the Bay of Bengal. Positive matrix factorization model was used for the source apportionment of the ionic species scavenged by rain. Comparable contributions of marine, dust, and anthropogenic sources were identified as major source over Kolkata. The major contributions were identified from marine and fossil fuel burning over Falta, whereas, marine, biomass/coal burning, ammonia from agricultural activities and domestic wastes were identified as the major sources over Darjeeling.

Dynamical model for the toroidal sporadic meteors

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pokorný, Petr; Vokrouhlický, David; Nesvorný, David

More than a decade of radar operations by the Canadian Meteor Orbit Radar have allowed both young and moderately old streams to be distinguished from the dispersed sporadic background component. The latter has been categorized according to broad radiant regions visible to Earth-based observers into three broad classes: the helion and anti-helion source, the north and south apex sources, and the north and south toroidal sources (and a related arc structure). The first two are populated mainly by dust released from Jupiter-family comets and new comets. Proper modeling of the toroidal sources has not to date been accomplished. Here, wemore » develop a steady-state model for the toroidal source of the sporadic meteoroid complex, compare our model with the available radar measurements, and investigate a contribution of dust particles from our model to the whole population of sporadic meteoroids. We find that the long-term stable part of the toroidal particles is mainly fed by dust released by Halley type (long period) comets (HTCs). Our synthetic model reproduces most of the observed features of the toroidal particles, including the most troublesome low-eccentricity component, which is due to a combination of two effects: particles' ability to decouple from Jupiter and circularize by the Poynting-Robertson effect, and large collision probability for orbits similar to that of the Earth. Our calibrated model also allows us to estimate the total mass of the HTC-released dust in space and check the flux necessary to maintain the cloud in a steady state.« less

Analysis of Light Absorbing Aerosols in Northern Pakistan: Concentration on Snow/Ice, their Source Regions and Impacts on Snow Albedo

NASA Astrophysics Data System (ADS)

Gul, C.; Praveen, P. S.; Shichang, K.; Adhikary, B.; Zhang, Y.; Ali, S.

2016-12-01

Elemental carbon (EC) and light absorbing organic carbon (OC) are important particulate impurities in snow and ice which significantly reduce the albedo of glaciers and accelerate their melting. Snow and ice samples were collected from Karakorum-Himalayan region of North Pakistan during the summer campaign (May-Jun) 2015 and only snow samples were collected during winter (Dec 2015- Jan 2016). Total 41 surface snow/ice samples were collected during summer campaign along different elevation ranges (2569 to 3895 a.m.s.l) from six glaciers: Sachin, Henarche, Barpu, Mear, Gulkin and Passu. Similarly 18 snow samples were collected from Sust, Hoper, Tawas, Astore, Shangla, and Kalam regions during the winter campaign. Quartz filters were used for filtering of melted snow and ice samples which were then analyzed by thermal optical reflectance (TOR) method to determine the concentration of EC and OC. The average concentration of EC (ng/g), OC (ng/g) and dust (ppm) were found as follows: Passu (249.5, 536.8, 475), Barpu (1190, 397.6, 1288), Gulkin (412, 793, 761), Sachin (911, 2130, 358), Mear (678, 2067, 83) and Henarche (755, 1868, 241) respectively during summer campaign. Similarly, average concentration of EC (ng/g), OC (ng/g) and dust (ppm) was found in the samples of Sust (2506, 1039, 131), Hoper (646, 1153, 76), Tawas (650, 1320, 16), Astore (1305, 2161, 97), Shangla (739, 2079, 31) and Kalam (107, 347, 5) respectively during winter campaign. Two methods were adopted to identify the source regions: one coupled emissions inventory with back trajectories, second with a simple region tagged chemical transport modeling analysis. In addition, CALIPSO subtype aerosol composition indicated that frequency of smoke in the atmosphere over the region was highest followed by dust and then polluted dust. SNICAR model was used to estimate the snow albedo reduction from our in-situ measurements. Snow albedo reduction was observed to be 0.3% to 27.6%. The derived results were used with SBDART clear sky solar fluxes to calculate the radiative forcing (RF). The RF values were observed to in the range of 0.43 to 36.75 W/m2 depending upon location.

Modern dust aerosol availability in northwestern China.

PubMed

Wang, Xunming; Cheng, Hong; Che, Huizheng; Sun, Jimin; Lu, Huayu; Qiang, Mingrui; Hua, Ting; Zhu, Bingqi; Li, Hui; Ma, Wenyong; Lang, Lili; Jiao, Linlin; Li, Danfeng

2017-08-18

The sources of modern dust aerosols and their emission magnitudes are fundamental for linking dust with climate and environment. Using field sample data, wind tunnel experiments and statistical analysis, we determined the contributions of wadis, gobi (stony desert), lakebeds, riverbeds, and interdunes to modern dust aerosol availability in the three important potential dust sources including the Tarim Basin, Qaidam Basin, and Ala Shan Plateau of China. The results show that riverbeds are the dominant landscape for modern dust aerosol availabilities in the Qaidam Basin, while wadis, gobi, and interdunes are the main landscapes over the Ala Shan Plateau and Tarim Basin. The Ala Shan Plateau and Tarim Basin are potential dust sources in northwestern China, while the Qaidam Basin is not a major source of the modern dust aerosols nowadays, and it is not acting in a significant way to the Loess Plateau presently. Moreover, most of modern dust aerosol emissions from China originated from aeolian processes with low intensities rather than from major dust events.

Two Molecular Clouds near M17

NASA Astrophysics Data System (ADS)

Wilson, T. L.; Hanson, M. M.; Muders, D.

2003-06-01

We present fully sampled images in the C18O J=2-1 line extending over 13'×23', made with the Heinrich Hertz Telescope (HHT) on Mount Graham, AZ. The HHT has a resolution of 35" at the line frequency. This region includes two molecular clouds. Cloud A, to the north, is more compact, while cloud B is to the west of the H II region M17. Cloud B contains the well-known source M17SW. In C18O we find 13 maxima in cloud A and 39 in cloud B. Sixteen sources in cloud B are in M17SW, mapped previously with higher resolution. In cloud B, sources outside M17SW have line widths comparable to those in M17SW. In comparison, cloud A has lower C18O line intensities and smaller line widths but comparable densities and sizes. Maps of the cores of these clouds were also obtained in the J=5-4 line of CS, which traces higher H2 densities. Our images of the cores of clouds A and B show that for VLSR<=20 km s-1, the peaks of the CS emission are shifted closer to the H II region than the C18O maxima, so higher densities are found toward the H II region. Our CS data give additional support to the already strong evidence that M17SW and nearby regions are heated and compressed by the H II region. Our data show that cloud A has a smaller interaction with the H II region. We surmise that M17SW was an initially denser region, and the turn-on of the H II region will make this the next region of massive star formation. Outside of M17SW, the only other obvious star formation region may be in cloud A, since there is an intense millimeter dust continuum peak found by Henning et al. (1998) but no corresponding C18O maximum. If the CO/H2 ratio is constant, the dust must have a temperature of ~100 K or the H2 density is greater than 106 cm-3 or both to reconcile the C18O and dust data. Alternatively, if the CO/H2 ratio is low, perhaps much of the CO is depleted.

Improved Dust Forecast Products for Southwest Asia Forecasters through Dust Source Database Advancements

NASA Astrophysics Data System (ADS)

Brooks, G. R.

2011-12-01

Dust storm forecasting is a critical part of military theater operations in Afghanistan and Iraq as well as other strategic areas of the globe. The Air Force Weather Agency (AFWA) has been using the Dust Transport Application (DTA) as a forecasting tool since 2001. Initially developed by The Johns Hopkins University Applied Physics Laboratory (JHUAPL), output products include dust concentration and reduction of visibility due to dust. The performance of the products depends on several factors including the underlying dust source database, treatment of soil moisture, parameterization of dust processes, and validity of the input atmospheric model data. Over many years of analysis, seasonal dust forecast biases of the DTA have been observed and documented. As these products are unique and indispensible for U.S. and NATO forces, amendments were required to provide the best forecasts possible. One of the quickest ways to scientifically address the dust concentration biases noted over time was to analyze the weaknesses in, and adjust the dust source database. Dust source database strengths and weaknesses, the satellite analysis and adjustment process, and tests which confirmed the resulting improvements in the final dust concentration and visibility products will be shown.

Laboratory study of PCB transport from primary sources to settled dust.

PubMed

Liu, Xiaoyu; Guo, Zhishi; Krebs, Kenneth A; Greenwell, Dale J; Roache, Nancy F; Stinson, Rayford A; Nardin, Joshua A; Pope, Robert H

2016-04-01

Dust is an important sink for indoor air pollutants, such as polychlorinated biphenyls (PCBs) that were used in building materials and products. In this study, two types of dust, house dust and Arizona Test Dust, were tested in a 30-m(3) stainless steel chamber with two types of panels. The PCB-containing panels were aluminum sheets coated with a PCB-spiked primer or caulk. The PCB-free panels were coated with the same materials but without PCBs. The dust evenly spread on each panel was collected at different times to determine its PCB content. The data from the PCB panels were used to evaluate the PCB migration from the source to the dust through direct contact, and the data from the PCB-free panels were used to evaluate the sorption of PCBs through the dust/air partition. Settled dust can adsorb PCBs from air. The sorption concentration was dependent on the congener concentration in the air and favored less volatile congeners. When the house dust was in direct contact with the PCB-containing panel, PCBs migrated into the dust at a much faster rate than the PCB transfer rate due to the dust/air partition. The dust/source partition was not significantly affected by the congener's volatility. For a given congener, the ratio between its concentration in the dust and in the source was used to estimate the dust/source partition coefficient. The estimated values ranged from 0.04 to 0.16. These values are indicative of the sink strength of the tested house dust being in the middle or lower-middle range. Published by Elsevier Ltd.

The impact of climate and composition on playa surface roughness: Investigation of atmospheric mineral dust emission mechanisms

NASA Astrophysics Data System (ADS)

Tollerud, H. J.; Fantle, M. S.

2011-12-01

Atmospheric mineral dust has a wide range of impacts, including the transport of elements in geochemical cycles, health hazards from small particles, and climate forcing via the reflection of sunlight from dust particles. In particular, the mineral dust component of climate forcing is one of the most uncertain elements in the IPCC climate forcing summary. Mineral dust is also an important component of geochemical cycles. For instance, dust inputs to the ocean potentially affect the iron cycle by stimulating natural iron fertilization, which could then modify climate via the biological pump. Also dust can transport nutrients over long distances and fertilize nutrient-poor regions, such as island ecosystems or the Amazon rain forest. However, there are still many uncertainties in quantifying dust emissions from source regions. One factor that influences dust emission is surface roughness and texture, since a weak, unconsolidated surface texture is more easily ablated by wind than a strong, hard crust. We are investigating the impact of processes such as precipitation, groundwater evaporation, and wind on surface roughness in a playa dust source region. We find that water has a significant influence on surface roughness. We utilize ESA's Advanced Synthetic Aperture Radar (ASAR) instrument to measure roughness in the playa. A map of roughness indicates where the playa surface is smooth (on the scale of centimeters) and potentially very strong, and where it is rough and might be more sensitive to disturbance. We have analyzed approximately 40 ASAR observations of the Black Rock Desert from 2007-2011. In general, the playa is smoother and more variable over time relative to nearby areas. There is also considerable variation within the playa. While the playa roughness maps changed significantly between summers and between observations during the winters, over the course of each summer, the playa surface maintained essentially the same roughness pattern. This suggests that there were no active processes during the summers that changed surface roughness. Images from NASA's MODIS instrument (1640 nm, band 6) delineate winter flooding on the playa. Areas of water in the winter tend to be smoother in the summer. In particular, a smooth area of the play in summer 2010 aligns very closely with ponded water in February 2010. This indicates that standing water disrupts the playa surface, reducing roughness. We also compared the distribution of surface roughness across the playa to playa composition. X-ray diffraction (XRD) of samples from the Black Rock Desert demonstrates that the playa surface is composed of approximately 30% quartz, 45% clays, 10% calcite, and 5% halite. Calcite and halite concentrations vary significantly between samples. We produced a map of calcite concentration in the Black Rock Desert based on hyperspectral data from NASA's EO-1 Hyperion instrument. We find that calcite concentrations are higher in smooth areas that have been inundated by water. Without an understanding of the surface processes associated with dust emission, it is difficult to model atmospheric dust, especially in the past or future when there is much less data for an empirical dust model.

Large-scale Desert Dust Deposition on the Himalayan Snow Cover: A Climatological Perspective from Satellite Observations

NASA Astrophysics Data System (ADS)

Gautam, R.; Hsu, N. C.; Lau, W. K.

2013-12-01

The Himalaya-Tibetan Plateau (HTP) has a profound influence on the Asian climate. The HTP are also among the largest snow/ice-covered regions on the Earth and provide major freshwater resource to the downstream densely-populated regions of Asia. Recent studies indicate climate warming over the HTP amplified by atmospheric heating and deposition of absorbing aerosols (e.g. dust and soot) over the HTP snowpack and glaciers. Recently, greater attention has focused on the effects of soot deposition on accelerated snowmelt and glacier retreat in the HTP, associated with increasing anthropogenic emissions in Asia. On the other hand, the role of transported dust affecting snow albedo/melt is not well understood over the HTP, in spite of the large annual cycle of mineral dust loading, particularly over the northern parts of south Asia during pre-monsoon season. This study addresses the large-scale effects of dust deposition on snow albedo in the elevated HTP from a satellite observational perspective. Dust aerosol transport, from southwest Asian arid regions, is observed in satellite imagery as darkening of the Himalayan snowpack. Additionally, multi-year spaceborne lidar observations, from CALIPSO, also show dust advected to elevated altitudes (~5km) over the Himalayan foothills, and episodically reaching the top of the western Himalaya. Spectral surface reflectance analysis of dust-laden snow cover (from MODIS) indicates enhanced absorption in the shorter visible wavelengths, yielding a significant gradient in the visible-nearIR reflectance spectrum. While soot in snow is difficult to distinguish from remote sensing, our spectral reflectance analysis of dust detection in the snowpack is consistent with theoretical simulations of snow darkening due to dust impurity. We find that the western HTP, in general, is influenced by enhanced dust deposition due to its proximity to major dust sources (and prevailing dust transport pathways), compared to the eastern HTP. Coinciding with the snowmelt period, dust deposition appears to further cause snow reflectance reduction, i.e. snow darkening, from spring to summer months. Among the entire HTP, we show that the western Himalaya and the Hindu-Kush snowpack are subjected to greater dust deposition and snow albedo reduction. Thus, our satellite-based observational study addresses the spatial variability of large-scale dust deposition on snow cover in the extensive HTP. A climatological and inter-annual perspective of the spatial variability of dust-induced snow darkening over the HTP will be presented, using ~10 years of MODIS spectral reflectance data (at high spatial resolution of ~1km). Results from this study provide insight into the particular role of desert dust towards accelerated seasonal snowmelt in the HTP.

Atmospheric inputs to watersheds of the Luquillo Mountains in eastern Puerto Rico: Chapter D in Water quality and landscape processes of four watersheds in eastern Puerto Rico

USGS Publications Warehouse

Stallard, Robert F.; Murphy, Sheila F.; Stallard, Robert F.

2012-01-01

Twenty years of precipitation-chemistry data from the National Atmospheric Deposition Program site at El Verde, Puerto Rico, demonstrate that three major sources control the composition of solutes in rain in eastern Puerto Rico. In order of importance, these sources are marine salts, temperate contamination from the Northern Hemisphere, and Sahara Desert dust. Marine salts are a source of roughly 82 percent of the ionic charge in precipitation; marine salt inputs are greatest in January. Evaluation of 15 years of U.S. Geological Survey data for four watersheds in eastern Puerto Rico suggests that large storms, including hurricanes, are associated with exceptionally high chloride concentrations in stream waters. Some of these storms were missed in sampling by the National Atmospheric Deposition Program, and therefore its data on the marine contribution likely underestimate chloride. The marine contribution is a weak source of acidity. Temperate contamination contributes about 10 percent of the ionic charge in precipitation; contaminants are primarily nitrate, ammonia, and sulfate derived from various manmade and natural sources. Peak deposition of temperate contaminants is during January, April, and May, months in which strong weather fronts arrive from the north. Temperate contamination, a strong source of acidity, is the only component that is increasing through time. Sahara Desert dust provides 5 percent of the ionic charge in precipitation; it is strongly seasonal, peaking in June and July during times of maximum dust transport from the Sahara and sub-Saharan regions. This dust contributes, on average, enough alkalinity to neutralize the acidity in June and July rains.

Tracing the Sources of Atmospheric Phosphorus Deposition to a Tropical Rain Forest in Panama Using Stable Oxygen Isotopes.

PubMed

Gross, A; Turner, B L; Goren, T; Berry, A; Angert, A

2016-02-02

Atmospheric dust deposition can be a significant source of phosphorus (P) in some tropical forests, so information on the origins and solubility of atmospheric P is needed to understand and predict patterns of forest productivity under future climate scenarios. We characterized atmospheric dust P across a seasonal cycle in a tropical lowland rain forest on Barro Colorado Nature Monument (BCNM), Republic of Panama. We traced P sources by combining remote sensing imagery with the first measurements of stable oxygen isotopes in soluble inorganic phosphate (δ(18)OP) in dust. In addition, we measured soluble inorganic and organic P concentrations in fine (<1 μm) and coarse (>1 μm) aerosol fractions and used this data to estimate the contribution of P inputs from dust deposition to the forest P budget. Aerosol dry mass was greater in the dry season (December to April, 5.6-15.7 μg m(-3)) than the wet season (May to November, 3.1-7.1 μg m(-3)). In contrast, soluble P concentrations in the aerosols were lower in the dry season (980-1880 μg P g(-1)) than the wet season (1170-3380 μg P g(-1)). The δ(18)OP of dry-season aerosols resembled that of nearby forest soils (∼19.5‰), suggesting a local origin. In the wet season, when the Trans-Atlantic Saharan dust belt moves north close to Panama, the δ(18)OP of aerosols was considerably lower (∼15.5‰), suggesting a significant contribution of long-distance dust P transport. Using satellite retrieved aerosol optical depth (AOD) and the P concentrations in aerosols we sampled in periods when Saharan dust was evident we estimate that the monthly P input from long distance dust transport during the period with highest Saharan dust deposition is 88 ± 31 g P ha(-1) month(-1), equivalent to between 10 and 29% of the P in monthly litter fall in nearby forests. These findings have important implications for our understanding of modern nutrient budgets and the productivity of tropical forests in the region under future climate scenarios.

A planetary dust ring generated by impact-ejection from the Galilean satellites

NASA Astrophysics Data System (ADS)

Sachse, Manuel

2018-03-01

All outer planets in the Solar System are surrounded by a ring system. Many of these rings are dust rings or they contain at least a high proportion of dust. They are often formed by impacts of micro-meteoroids onto embedded bodies. The ejected material typically consists of micron-sized charged particles, which are susceptible to gravitational and non-gravitational forces. Generally, detailed information on the dynamics and distribution of the dust requires expensive numerical simulations of a large number of particles. Here we develop a relatively simple and fast, semi-analytical model for an impact-generated planetary dust ring governed by the planet's gravity and the relevant perturbation forces for the dynamics of small charged particles. The most important parameter of the model is the dust production rate, which is a linear factor in the calculation of the dust densities. We apply our model to dust ejected from the Galilean satellites using production rates obtained from flybys of the dust sources. The dust densities predicted by our model are in good agreement with numerical simulations and with in situ measurements by the Galileo spacecraft. The lifetimes of large particles are about two orders of magnitude greater than those of small ones, which implies a flattening of the size distribution in circumplanetary space. Information about the distribution of circumplanetary dust is also important for the risk assessment of spacecraft orbits in the respective regions.

Type-segregated aerosol effects on regional monsoon activity: A study using ground-based experiments and model simulations

NASA Astrophysics Data System (ADS)

Vijayakumar, K.; Devara, P. C. S.; Sonbawne, S. M.

2014-12-01

Classification of observed aerosols into key types [e.g., clean-maritime (CM), desert-dust (DD), urban-industrial/biomass-burning (UI/BB), black carbon (BC), organic carbon (OC) and mixed-type aerosols (MA)] would facilitate to infer aerosol sources, effects, and feedback mechanisms, not only to improve the accuracy of satellite retrievals but also to quantify the assessment of aerosol radiative impacts on climate. In this paper, we report the results of a study conducted in this direction, employing a Cimel Sun-sky radiometer at the Indian Institute of Tropical Meteorology (IITM), Pune, India during 2008 and 2009, which represent two successive contrasting monsoon years. The study provided an observational evidence to show that the local sources are subject to heavy loading of absorbing aerosols (dust and black carbon), with strong seasonality closely linked to the monsoon annual rainfall cycle over Pune, a tropical urban station in India. The results revealed the absence of CM aerosols in the pre-monsoon as well as in the monsoon seasons of 2009 as opposed to 2008. Higher loading of dust aerosols is observed in the pre-monsoon and monsoon seasons of 2009; majority may be coated with fine BC aerosols from local emissions, leading to reduction in regional rainfall. Further, significant decrease in coarse-mode AOD and presence of carbonaceous aerosols, affecting the aerosol-cloud interaction and monsoon-rain processes via microphysics and dynamics, is considered responsible for the reduction in rainfall during 2009. Additionally, we discuss how optical depth, contributed by different types of aerosols, influences the distribution of monsoon rainfall over an urban region using the Monitoring Atmospheric Composition and Climate (MACC) aerosol reanalysis. Furthermore, predictions of the Dust REgional Atmospheric Model (DREAM) simulations combined with HYSPLIT (HYbrid Single Particle Lagrangian Integrated Trajectory) cluster model are also discussed in support of the observed features.

Contribution of dust storms to PM10 levels in an urban arid environment.

PubMed

Krasnov, Helena; Katra, Itzhak; Koutrakis, Petros; Friger, Michael D

2014-01-01

Quantitative information on the contribution of dust storms to atmospheric PM10 (particulate matter with an aerodynamic diameter < or = 10 microm) levels is still lacking, especially in urban environments with close proximity to dust sources. The main objective of this study was to quantify the contribution of dust storms to PM10 concentrations in a desert urban center, the city of Beer-Sheva, Negev, Israel, during the period of 2001-2012. Toward this end, a background value based on the "dust-free" season was used as a threshold value to identify potentially "dust days." Subsequently, the net contribution of dust storms to PM10 was assessed. During the study period, daily PM10 concentrations ranged from 6 to over 2000 microg/m3. In each year, over 10% of the daily concentrations exceeded the calculated threshold (BVt) of 71 microg/m3. An average daily net contribution of dust to PM10 of 122 microg/m3 was calculated for the entire study period based on this background value. Furthermore, a dust storm intensity parameter (Ai) was used to analyze several storms with very high PM10 contributions (hourly averages of 1000-5197 microg/m3). This analysis revealed that the strongest storms occurred mainly in the last 3 yr of the study. Finally, these findings indicate that this arid urban environment experiences high PM10 levels whose origin lies in both local and regional dust events. The findings indicate that over time, the urban arid environment experiences high PM10 levels whose origin lies in local and regional dust events. It was noticed that the strongest storms have occurred mainly in the last 3 yr. It is believed that environmental changes such as global warming and desertification may lead to an increased air pollution and risk exposure to human health.

Millennial-scale fluctuations in Saharan dust supply across the decline of the African Humid Period

NASA Astrophysics Data System (ADS)

Zielhofer, Christoph; von Suchodoletz, Hans; Fletcher, William J.; Schneider, Birgit; Dietze, Elisabeth; Schlegel, Michael; Schepanski, Kerstin; Weninger, Bernhard; Mischke, Steffen; Mikdad, Abdeslam

2017-09-01

The Sahara is the world's largest dust source with significant impacts on trans-Atlantic terrestrial and large-scale marine ecosystems. Contested views about a gradual or abrupt onset of Saharan aridity at the end of the African Humid Period dominate the current scientific debate about the Holocene Saharan desiccation. In this study, we present a 19.63 m sediment core sequence from Lake Sidi Ali (Middle Atlas, Morocco) at the North African desert margin. We reconstruct the interaction between Saharan dust supply and Western Mediterranean hydro-climatic variability during the last 12,000 yr based on analyses of lithogenic grain-sizes, XRF geochemistry and stable isotopes of ostracod shells. A robust chronological model based on AMS 14C dated pollen concentrates supports our multi-proxy study. At orbital-scale there is an overall increase in southern dust supply from the Early Holocene to the Late Holocene, but our Northern Saharan dust record indicates that a gradual Saharan desiccation was interrupted by multiple abrupt dust increases before the 'southern dust mode' was finally established at 4.7 cal ka BP. The Sidi Ali record features millennial peaks in Saharan dust increase at about 11.1, 10.2, 9.4, 8.2, 7.3, 6.6, 6.0, and 5.0 cal ka BP. Early Holocene Saharan dust peaks coincide with Western Mediterranean winter rain minima and North Atlantic cooling events. In contrast, Late Holocene dust peaks correspond mostly with prevailing positive phases of the North Atlantic Oscillation. By comparing with other North African records, we suggest that increases in Northern Saharan dust supply do not solely indicate sub-regional to regional aridity in Mediterranean Northwest Africa but might reflect aridity at a trans-Saharan scale. In particular, our findings support major bimillennial phases of trans-Saharan aridity at 10.2, 8.2, 6.0 and 4.2 cal ka BP. These phases coincide with North Atlantic cooling and a weak African monsoon.

Surface Measurements of dust/local aerosol properties over Northern China during 2008 China-US joined dust field campaign

NASA Astrophysics Data System (ADS)

Wang, X.; Huang, J.

2009-12-01

The objective of this study is to understand the detailed characteristics and underlying mechanisms of aerosol physical and optical parameters over China Loess Plateau and its potential impacts on the regional/global climate. In order to characterize the emission, transport, and removal of atmospheric pollutants emitted from East Asia, the 2008 China-US joined field campaign are conducted from late April to May 2008 focused specifically on the Asian direct measurements of dust and pollution transport, following the plume from the Northern China which from the Taklamakan desert and Gobi desert to the Eastern Pacific and into North America. Such measurements are crucial to understanding how the dust and the pollution plume (including black carbon) are modified as their age. Three sites involved this campaign, including one permanent site (Semi-Arid Climate & Environment Observatory of Lanzhou University (SACOL)) (located in Yuzhong, 35.95N/104.1E), one SACOL's Mobile Facility (SMF) (deployed in Jintai, 37.57N/104.23E) and the U.S. Department of Energy Atmospheric Radiation Measurements(ARM) Ancillary Facility (AAF mobile laboratories, SMART-COMMIT) (deployed in Zhangye, 39.08N/100.27E). Results indicate that the dust plumes are transported from the surface to a long distance from their sources have a significant influence on the air quality in the study area. The meteorological analysis indicates that these polluted layers are not from local sources during dust plume and this large-scale transport of dust and pollutants remains a major uncertainty in quantifying the global effect of emissions from Northern China.

Characterization of Saharan mineral dust transported to the Colle Gnifetti glacier (Southern Alps, Switzerland) during the last centuries.

NASA Astrophysics Data System (ADS)

Thevenon, Florian; Poté, John; Adatte, Thierry; Chiaradia, Massimo; Hueglin, Christoph; Collaud Coen, Martine

2010-05-01

The Southern Alps act as a barrier to the southwesterly dust-laden winds from the Sahara, and the Colle Gnifetti saddle (45°55'N, 7°52'E, 4455 m asl in the Monte Rosa Massif) satisfactory conserves the history of climatic conditions over the last millennium (Thevenon et al., 2009). Therefore, the Colle Gnifetti glacier is a suitable site for i) studying the composition of past Saharan aeolian dust emissions, and for ii) comparing modern dust emissions with preindustrial emissions. The mineral aerosols entrapped in the ice core have been analyzed for their physical (grain-size by image analysis), mineralogical (by X-ray diffraction), and chemical composition (by ICPMS and by mass spectrometry for Sr and Nd isotopic ratios). The mineral dust characteristics are then compared with present day Saharan dust samples collected at the high altitude research station Jungfraujoch (46°55'N, 7°98E, 3580 asl) and with documented potential dust sources. Results show that i) the increases in atmospheric dustiness correlate with larger mean grain size, and that ii) the dust emissions increase after the industrial revolution, probably as a large-scale atmospheric circulation response to anthropogenic climate forcing (Shindell et al., 2001; Thevenon et al., 2009). However, geochemical variations in aeolian mineral particles also indicate that the source areas of the dust, which are now situated in northern and north-western part of the Saharan desert (Collaud Coen et al., 2004), did not change significantly throughout the past. Therefore, the mineralogy (e.g. illite, kaolinite, chlorite, palygorskite) and the geochemistry of the paleo-dust particles transported to Europe, are relevant to assess past African dust sources. REFERENCES: - Thevenon, F., F. S. Anselmetti, S. M. Bernasconi, and M. Schwikowski (2009). Mineral dust and elemental black carbon records from an Alpine ice core (Colle Gnifetti glacier) over the last millennium. J. Geophys. Res., 114, D17102, doi:10.1029/2008JD011490. - Collaud Coen, M., E. Weingartner, D. Schaub, C. Hueglin, C. Corrigan, S. Henning, M. Schwikowski, and U. Baltensperger (2004), Saharan dust events at the Jungfraujoch: Detection by wavelength dependence of the single scattering albedo and first climatology analysis, Atmos. Chem. Phys., 4, 2465- 2480. - Shindell, D. T., G. A. Schmidt, M. E. Mann, D. Rind, and A. Waple (2001). Solar forcing of regional climate change during the Maunder Minimum, Science, 294, 2149-2152, doi:10.1126/science.1064363.

Physical and chemical properties of deposited airborne particulates over the Arabian Red Sea coastal plain

NASA Astrophysics Data System (ADS)

Engelbrecht, Johann P.; Stenchikov, Georgiy; Jish Prakash, P.; Lersch, Traci; Anisimov, Anatolii; Shevchenko, Illia

2017-09-01

Mineral dust is the most abundant aerosol, having a profound impact on the global energy budget. This research continues our previous studies performed on surface soils in the Arabian Peninsula, focusing on the mineralogical, physical and chemical composition of dust deposits from the atmosphere at the Arabian Red Sea coast. For this purpose, aerosols deposited from the atmosphere are collected during 2015 at six sites on the campus of the King Abdullah University of Science and Technology (KAUST) situated on the Red Sea coastal plain of Saudi Arabia and subjected to the same chemical and mineralogical analysis we conducted on soil samples. Frisbee deposition samplers with foam inserts were used to collect dust and other deposits, for the period December 2014 to December 2015. The average deposition rate measured at KAUST for this period was 14 g m-2 per month, with lowest values in winter and increased deposition rates in August to October. The particle size distributions provide assessments of < 10 and < 2.5 µm dust deposition rates, and it is suggested that these represent proxies for PM10 (coarse) and PM2. 5 (fine) particle size fractions in the dust deposits.X-ray diffraction (XRD) analysis of a subset of samples confirms variable amounts of quartz, feldspars, micas, and halite, with lesser amounts of gypsum, calcite, dolomite, hematite, and amphibole. Freeze-dried samples were re-suspended onto the Teflon® filters for elemental analysis by X-ray fluorescence (XRF), while splits from each sample were analyzed for water-soluble cations and anions by ion chromatography. The dust deposits along the Red Sea coast are considered to be a mixture of dust emissions from local soils and soils imported from distal dust sources. Airborne mineral concentrations are greatest at or close to dust sources, compared to those through medium- and long-range transport. It is not possible to identify the exact origin of deposition samples from the mineralogical and chemical results alone. These aerosol data are the first of their kind from the Red Sea region. They will help assess their potential nutrient input into the Red Sea, as well the impact on human health, industry, and solar panel efficiency. These data will also support dust modeling in this important dust belt source area by better quantifying dust mass balance and optical properties of airborne dust particles.

Dust grains from the heart of supernovae

NASA Astrophysics Data System (ADS)

Bocchio, M.; Marassi, S.; Schneider, R.; Bianchi, S.; Limongi, M.; Chieffi, A.

2016-03-01

Dust grains are classically thought to form in the winds of asymptotic giant branch (AGB) stars. However, there is increasing evidence today for dust formation in supernovae (SNe). To establish the relative importance of these two classes of stellar sources of dust, it is important to know the fraction of freshly formed dust in SN ejecta that is able to survive the passage of the reverse shock and be injected in the interstellar medium. With this aim, we have developed a new code, GRASH_Rev, that allows following the dynamics of dust grains in the shocked SN ejecta and computing the time evolution of the mass, composition, and size distribution of the grains. We considered four well-studied SNe in the Milky Way and Large Magellanic Cloud: SN 1987A, CasA, the Crab nebula, and N49. These sources have been observed with both Spitzer and Herschel, and the multiwavelength data allow a better assessment the mass of warm and cold dust associated with the ejecta. For each SN, we first identified the best explosion model, using the mass and metallicity of the progenitor star, the mass of 56Ni, the explosion energy, and the circumstellar medium density inferred from the data. We then ran a recently developed dust formation model to compute the properties of freshly formed dust. Starting from these input models, GRASH_Rev self-consistently follows the dynamics of the grains, considering the effects of the forward and reverse shock, and allows predicting the time evolution of the dust mass, composition, and size distribution in the shocked and unshocked regions of the ejecta. All the simulated models aagree well with observations. Our study suggests that SN 1987A is too young for the reverse shock to have affected the dust mass. Hence the observed dust mass of 0.7-0.9 M⊙ in this source can be safely considered as indicative of the mass of freshly formed dust in SN ejecta. Conversely, in the other three SNe, the reverse shock has already destroyed between 10-40% of the initial dust mass. However, the largest dust mass destruction is predicted to occur between 103 and 105 yr after the explosions. Since the oldest SN in the sample has an estimated age of 4800 yr, current observations can only provide an upper limit to the mass of SN dust that will enrich the interstellar medium, the so-called effective dust yields. We find that only between 1-8% of the currently observed mass will survive, resulting in an average SN effective dust yield of (1.55 ± 1.48) × 10-2M⊙. This agrees well with the values adopted in chemical evolution models that consider the effect of the SN reverse shock. We discuss the astrophysical implications of our results for dust enrichment in local galaxies and at high redshift.

Climate change and the collapse of the Akkadian empire: Evidence from the deep sea

NASA Astrophysics Data System (ADS)

Cullen, H. M.; Demenocal, P. B.; Hemming, S.; Hemming, G.; Brown, F. H.; Guilderson, T.; Sirocko, F.

2000-04-01

The Akkadian empire ruled Mesopotamia from the headwaters of the Tigris-Euphrates Rivers to the Persian Gulf during the late third millennium B.C. Archeological evidence has shown that this highly developed civilization collapsed abruptly near 4170 ± 150 calendar yr B.P., perhaps related to a shift to more arid conditions. Detailed paleoclimate records to test this assertion from Mesopotamia are rare, but changes in regional aridity are preserved in adjacent ocean basins. We document Holocene changes in regional aridity using mineralogic and geochemical analyses of a marine sediment core from the Gulf of Oman, which is directly downwind of Mesopotamian dust source areas and archeological sites. Our results document a very abrupt increase in eolian dust and Mesopotamian aridity, accelerator mass spectrometer radiocarbon dated to 4025 ± 125 calendar yr B.P., which persisted for ˜300 yr. Radiogenic (Nd and Sr) isotope analyses confirm that the observed increase in mineral dust was derived from Mesopotamian source areas. Geochemical correlation of volcanic ash shards between the archeological site and marine sediment record establishes a direct temporal link between Mesopotamian aridification and social collapse, implicating a sudden shift to more arid conditions as a key factor contributing to the collapse of the Akkadian empire.

High-contrast imaging of HD 163296 with the Keck/NIRC2 L΄-band vortex coronograph

NASA Astrophysics Data System (ADS)

Guidi, G.; Ruane, G.; Williams, J. P.; Mawet, D.; Testi, L.; Zurlo, A.; Absil, O.; Bottom, M.; Choquet, É.; Christiaens, V.; Castellá, B. Femenía; Huby, E.; Isella, A.; Kastner, J.; Meshkat, T.; Reggiani, M.; Riggs, A.; Serabyn, E.; Wallack, N.

2018-06-01

We present observations of the nearby (D˜100 pc) Herbig star HD 163296 taken with the vortex coronograph at Keck/NIRC2 in the L' band (3.7 μm), to search for planetary mass companions in the ringed disc surrounding this pre-main sequence star. The images reveal an arc-like region of scattered light from the disc surface layers that is likely associated with the first bright ring detected with ALMA in the λ=1.3mm dust continuum at ˜65 au. We also detect a point-like source at ˜0{^''.}5 projected separation in the North-East direction, close to the inner edge of the second gap in the millimetre images. Comparing the point source photometry with the atmospheric emission models of non-accreting giant planets, we obtain a mass of 6-7 MJ for a putative protoplanet, assuming a system age of 5 Myr. Based on the contrast at a 95% level of completeness calculated on the emission-free regions of our images, we set upper limits for the masses of giant planets of 8-15 MJ, 4.5-6.5 MJ and 2.5-4.0 MJ at the locations of the first, second and third gap in the millimetre dust continuum, respectively. Further deep, high resolution thermal IR imaging of the HD 163296 system are warranted, to confirm the presence and nature of the point source and to better understand the structure of the dust disc.

The effects of dust on Colorado mountain snow cover albedo and compositional links to dust-source areas

NASA Astrophysics Data System (ADS)

Goldstein, H. L.; Reynolds, R. L.; Landry, C.; Derry, J. E.; Kokaly, R. F.; Breit, G. N.

2016-12-01

Dust deposited on mountain snow cover (DOS) changes snow albedo, enhances absorption of solar radiation, and effectively increases rates of snow melt, leading to earlier-than-normal runoff and overall smaller late-season water supplies for tens of millions of people and industries in the American West. Visible-spectrum reflectance of DOS samples is on the order of 0.2 (80% absorption), in stark contrast to the high reflectivity of pure snow which approaches 1.0. Samples of DOS were collected from 12 high-elevation Colorado mountain sites near the end of spring from 2013 through 2016 prior to complete snow melt, when most dust layers had merged into one layer. These samples were analyzed to measure dust properties that affect snow albedo and to link DOS to dust-source areas. Dust mass loadings to snow during water year 2014 varied from 5 to 30 g/m2. Median particle sizes centered around 20 micrometers with more than 80% of the dust <63 micrometers. Dark minerals, carbonaceous matter, and iron oxides, including nano-sized hematite and goethite, together diminished reflectance according to their variable concentrations. Documenting variations in dust-particle masses, sizes, and compositions helps determine their influences on snow-melt and may be useful for modeling snow-melt effects from future dust. Furthermore, variations in dust components and particle sizes lead to new ways to recognize sources of dust by comparison with properties of fine-grained sediments in dust-source areas. Much of the DOS in the San Juan Mountains, Colorado can be linked to southern Colorado Plateau source areas by compositional similarities and satellite imagery. Understanding dust properties that affect snow albedo and recognizing the sources of dust deposited on snow cover may guide mitigation of dust emission that affects water resources of the Colorado River basin.

Earth Observations taken by the Expedition 17 Crew

NASA Image and Video Library

2008-10-16

ISS017-E-019616 (16 Oct. 2008) --- A dust storm in Turkmenistan, Central Asia is featured in this image photographed by an Expedition 17 crewmember on the International Space Station. This west-looking view, taken with a short focal length lens from the station, shows a wide swath of central Asia--from Afghanistan, along the length of Turkmenistan to the Caspian Sea. Winds blowing down the largest river valley in the region, the Amudarya, were strong enough to raise a large dust storm. Dust appears as a light brown mass extending into the center of the image from the lower right. Diffuse dust from prior windy weather appears over much of the area making a regional haze that clouds much of the landscape detail. The haze partly obscures the irrigated agriculture in Turkmenistan and entirely obscures the Caspian Sea. Numerous rivers rise in the Hindu Kush mountain complex (lower left). The Band-i Amir River is a major tributary of the main regional river, the Amudarya, which it reaches via a deep canyon. The Amudarya River was the major historical contributor of water to the Aral Sea, but today extensive diversion of river water for agricultural purposes has lead to extensive exposure and desiccation of the sea bed. The exposed sea bed is a major source of saline dusts contaminated with agricultural chemicals that pose a significant environmental hazard to central Asia. To a lesser extent, dusts are also mobilized from sediments along the Amudarya river channel. The Paropamisus Range and the Amudarya (also known as the Oxus River) are mentioned in histories of Alexander the Great's famous military expedition from Greece to India. His horsemen made a fast side excursion from near the Caspian Sea (top right) as far as the Amudarya (lower right).

Using dust, gas and stellar mass-selected samples to probe dust sources and sinks in low-metallicity galaxies

NASA Astrophysics Data System (ADS)

De Vis, P.; Gomez, H. L.; Schofield, S. P.; Maddox, S.; Dunne, L.; Baes, M.; Cigan, P.; Clark, C. J. R.; Gomez, E. L.; Lara-López, M.; Owers, M.

2017-10-01

We combine samples of nearby galaxies with Herschel photometry selected on their dust, metal, H I and stellar mass content, and compare these to chemical evolution models in order to discriminate between different dust sources. In a companion paper, we used an H I-selected sample of nearby galaxies to reveal a subsample of very gas-rich (gas fraction >80 per cent) sources with dust masses significantly below predictions from simple chemical evolution models, and well below Md/M* and Md/Mgas scaling relations seen in dust and stellar-selected samples of local galaxies. We use a chemical evolution model to explain these dust-poor, but gas-rich, sources as well as the observed star formation rates (SFRs) and dust-to-gas ratios. We find that (I) a delayed star formation history is required to model the observed SFRs; (II) inflows and outflows are required to model the observed metallicities at low gas fractions; (III) a reduced contribution of dust from supernovae (SNe) is needed to explain the dust-poor sources with high gas fractions. These dust-poor, low stellar mass galaxies require a typical core-collapse SN to produce 0.01-0.16 M⊙ of dust. To match the observed dust masses at lower gas fractions, significant grain growth is required to counteract the reduced contribution from dust in SNe and dust destruction from SN shocks. These findings are statistically robust, though due to intrinsic scatter it is not always possible to find one single model that successfully describes all the data. We also show that the dust-to-metal ratio decreases towards lower metallicity.

Mass closure and source apportionment of PM2.5 by Positive Matrix Factorization analysis in urban Mediterranean environment

NASA Astrophysics Data System (ADS)

Mantas, E.; Remoundaki, E.; Halari, I.; Kassomenos, P.; Theodosi, C.; Hatzikioseyian, A.; Mihalopoulos, N.

2014-09-01

A systematic monitoring of PM2.5 was carried out during a period of three years (from February 2010 to April 2013) at an urban site, at the National Technical University of Athens campus. Two types of 24-h PM2.5 samples have been collected: 271 samples on PTFE and 116 samples on quartz filters. Daily PM2.5 concentrations were determined for both types of samples. Total sulfur, crustal origin elements and elements of a major crustal component (Al, Si, Fe, Ca, K, Mg, Ti) trace elements (Zn, Pb, Cu, Ni, P, V, Cr, Mn) and water soluble ions (Cl-, NO3-, SO42-, Na+, K+, NH4+, Ca2+, Mg2+) were determined on the PTFE samples. Organic carbon (OC), elemental carbon (EC) and water soluble ions were determined on the quartz samples. For the mass closure six components were considered: Secondary Inorganic Aerosol (SIA), Organic Matter (OM), Elemental Carbon (EC), Dust, Mineral anthropogenic component (MIN) and Sea Salt (SS). SIA and OM contributed in the mass of PM2.5 almost equally: 30-36% and 30% respectively. EC, SS and MIN accounted for 5, 4 and 3% respectively of the total PM2.5 mass. Dust accounted for about 3-5% in absence of dust transport event and reached a much higher percentage in case of dust transport event. These contributions justify at least 80% of the PM2.5 mass. Source apportionment analysis has been performed by Positive Matrix Factorization. The combination of the PMF results obtained by both data sets lead to the definition of six factors: 1. SO42-, NH4+, OC (industrial/regional sources, secondary aerosol) 2. EC, OC, K and trace metals (traffic and heating by biomass burning, locally emitted aerosol). 3. Ca, EC, OC and trace metals (urban-resuspended road dust reflecting exhaust emissions), 4. Secondary nitrates 5. Na, Cl (marine source) 6. Si, Al, Ti, Ca, Fe (Dust transported from Sahara). These factors reflect not only main sources contributions but also underline the key role of atmospheric dynamics and aerosol ageing processes in this Mediterranean environment.

Distribution of pesticides in dust particles in urban environments.

PubMed

Richards, Jaben; Reif, Ruben; Luo, Yuzhuo; Gan, Jay

2016-07-01

In regions with a mild climate, pesticides are often used around homes for pest control. Recent monitoring studies have linked pesticide use in residential areas to aquatic toxicity in urban surface water ecosystems, and suggested dust particles on paved surfaces as an important source of pesticides. To test the hypothesis that dust on hard surfaces is a significant source of pesticides, we evaluated spatial and temporal patterns of current-use insecticides in Southern California, and further explored their distribution as a function of particle sizes. Pyrethroid insecticides were detected in dust from the driveway, curb gutter and street at 53.5-94.8%, with median concentrations of 1-46 ng g(-1). Pyrethroid residues were uniformly distributed in areas adjacent to a house, suggesting significant redistribution. The total levels of pyrethroids in dust significantly (p < 0.01) decreased from October to February, suggesting rainfalls as a major mechanism to move pesticide residues offsite. Fipronil as well as its degradation products, were detected at 50.6-75.5%, and spatial and temporal patterns of fipronil residues suggested rapid transformations of fipronil to its biologically active intermediates. Moreover, pyrethroids were found to be enriched in fine particles that have a higher mobility in runoff than coarse particles. Results from this study highlight the widespread occurrence of pesticides in outdoor dust around homes and the potential contribution to downstream surface water contamination via rain-induced runoff. Copyright © 2016 Elsevier Ltd. All rights reserved.

PAHs underfoot: contaminated dust from coal-tar sealcoated pavement is widespread in the United States

DOE Office of Scientific and Technical Information (OSTI.GOV)

Peter C. Van Metre; Barbara J. Mahler; Jennifer T. Wilson

We reported in 2005 that runoff from parking lots treated with coal-tar-based sealcoat was a major source of polycyclic aromatic hydrocarbons (PAHs) to streams in Austin, Texas. Here we present new data from nine U.S. cities that show nationwide patterns in concentrations of {Sigma}PAHs associated with sealcoat. Dust was swept from parking lots in six cities in the central and eastern U.S., where coal-tar-based sealcoat dominates use, and three cities in the western U.S., where asphalt-based sealcoat dominates use. For six central and eastern cities, median SPAH concentrations in dust from sealcoated and unsealcoated pavement are 2200 and 27 mg/kg,more » respectively. For three western cities, median SPAH concentrations in dust from sealcoated and unsealcoated pavement are similar and very low (2.1 and 0.8 mg/kg, respectively). Lakes in the central and eastern cities where pavement was sampled have bottom sediments with higher PAH concentrations than do those in the western cities relative to degree of urbanization. Bottom-sediment PAH assemblages are similar to those of sealcoated pavement dust regionally, implicating coal-tar-based sealcoat as a PAH source to the central and eastern lakes. Concentrations of benzo(a)pyrene in dust from coal-tar sealcoated pavement and adjacent soils greatly exceed generic soil screening levels, suggesting that research on human-health risk is warranted. 30 refs., 4 figs., 2 tabs.« less

Petrogenic organic carbon and PAHs in snow deposited on Athabasca oil sands region lakes

NASA Astrophysics Data System (ADS)

Ahad, J. M.; Pakdel, H.; Gammon, P. R.; Savard, M. M.

2017-12-01

Fugitive dust associated with surface mining activities is one of the principal vectors for transport of airborne contaminants in Canada's Athabasca oil sands (AOS) region. The two main sources for mining-related dust - unprocessed oil sand and petroleum coke (petcoke) - contain high levels of bitumen-derived organic contaminants such as polycyclic aromatic hydrocarbons (PAHs). Here, we report the radiocarbon (14C) contents of solvent-extractable organics in snow particulates deposited during the winter of 2016-17 on fourteen lakes across the AOS region to quantify the contribution of anthropogenic dust transported directly to these ecosystems. Concentrations of parent and alkylated PAHs were determined in both dissolved and particulate fractions of snow. Radiocarbon isotope ratios (Δ14C) ranged from -805 to -177‰, indicating a significant contribution of petrogenic or fossil (i.e., Δ14C = -1000‰) carbon in snowpack dust at some sites. More negative Δ14C values were generally found in samples containing higher levels of particulate matter and at lakes closer to the geographic center of AOS mining operations. Concentrations of PAHs > 2 rings were significantly higher in the particulate phase and in samples with the largest petrogenic carbon components. Relatively high levels of PAHs at some distal sites associated with less negative Δ14C values pointed to an important modern carbon contribution, potentially ash originating from the 1.5 million acre 2016 Fort McMurray wildfire. As demonstrated here, fugitive dust in snow covering AOS region lakes can contain significant petrogenic organic carbon and high levels of PAHs, particularly in areas close (i.e., < 25 km) to the center of AOS mining operations. The spring snowmelt thus provides a direct pathway for mining-related contaminants to lake sediments.

Seasonal variations in the sources of natural and anthropogenic lead deposited at the East Rongbuk Glacier in the high-altitude Himalayas.

PubMed

Burn-Nunes, Laurie; Vallelonga, Paul; Lee, Khanghyun; Hong, Sungmin; Burton, Graeme; Hou, Shugui; Moy, Andrew; Edwards, Ross; Loss, Robert; Rosman, Kevin

2014-07-15

Lead (Pb) isotopic compositions and concentrations, and barium (Ba) and indium (In) concentrations have been analysed at sub-annual resolution in three sections from a <110 m ice core dated to the 18th and 20th centuries, as well as snow pit samples dated to 2004/2005, recovered from the East Rongbuk Glacier in the high-altitude Himalayas. Ice core sections indicate that atmospheric chemistry prior to ~1,953 was controlled by mineral dust inputs, with no discernible volcanic or anthropogenic contributions. Eighteenth century monsoon ice core chemistry is indicative of dominant contributions from local Himalayan sources; non-monsoon ice core chemistry is linked to contributions from local (Himalayan), regional (Indian/Thar Desert) and long-range (North Africa, Central Asia) sources. Twentieth century monsoon and non-monsoon ice core data demonstrate similar seasonal sources of mineral dust, however with a transition to less-radiogenic isotopic signatures that suggests local and regional climate/environmental change. The snow pit record demonstrates natural and anthropogenic contributions during both seasons, with increased anthropogenic influence during non-monsoon times. Monsoon anthropogenic inputs are most likely sourced to South/South-East Asia and/or India, whereas non-monsoon anthropogenic inputs are most likely sourced to India and Central Asia. Copyright © 2014 Elsevier B.V. All rights reserved.

Temporal Dynamics of Sodic Playa Salt Crust Patterns: Implications for Aeolian Dust Emission Potential

NASA Astrophysics Data System (ADS)

Nield, J. M.; King, J.; Bryant, R. G.; Wiggs, G.; Eckardt, F. D.; Thomas, D. S.; Washington, R.

2013-12-01

Salt pans (or playas) are common in arid environments and can be major sources of windblown mineral dust, but there are uncertainties associated with their dust emission potential. These landforms typically form crusts which modify both their erosivity and erodibility by limiting sediment availability, modifying surface and aerodynamic roughness and limiting evaporation rates and sediment production. Here we show the relationship between seasonal surface moisture change and crust pattern development based on both remote-sensing and field surface and atmospheric measurements. We use high resolution (sub-cm) terrestrial laser scanning (TLS; ground-based lidar) surveys over weekly, monthly and annual timescales to accurately characterise crustal ridge thrusting and collapse. This can be as much as 2 mm/day on fresh pan areas that have recently been reset by flooding. Over a two month period, this ridge growth can change aerodynamic roughness length values by 6.5 mm. At the same time, crack densities across the surface increase and this raises the availability of erodible fluffy, low density dust source sediment stored below the crust layer. Ridge spaces are defined in the early stages of crust development, as identified by Fourier Transform analysis, but wider wavelengths become more pronounced over time. We present a conceptual model accounting for the driving forces (subsurface, surface and atmospheric moisture) and feedbacks between these and surface shape that lead to crust pattern trajectories between highly emissive degraded surfaces and less emissive ridged or continuous crusts. These findings improve our understanding of temporal changes in dust availability and supply from playa source regions.

[Distribution Characteristics and Source Analysis of Dustfall Trace Elements During Winter in Beijing].

PubMed

Xiong, Qiu-lin; Zhao, Wen-ji; Guo, Xiao-yu; Chen, Fan-tao; Shu, Tong-tong; Zheng, Xiao-xia; Zhao, Wen-hui

2015-08-01

The dustfall content is one of the evaluation indexes of atmospheric pollution. Trace elements especially heavy metals in dustfall can lead to risks to ecological environment and human health. In order to study the distribution characteristics of trace elements, heavy metals pollution and their sources in winter atmospheric dust, 49 dustfall samples were collected in Beijing City and nearby during November 2013 to March 2014. Then the contents (mass percentages) of 40 trace elements were measured by Elan DRC It type inductively coupled plasma mass (ICP-MS). Test results showed that more than half of the trace elements in the dust were less than 10 mg x kg(-1); about a quarter were between 10-100 mg x kg-1); while 7 elements (Pb, Zr, Cr, Cu, Zn, Sr and Ba) were more than 100 mg x kg(-1). The contents of Pb, Cu, Zn, Bi, Cd and Mo of winter dustfall in Beijing city.were respectively 4.18, 4.66, 5.35, 6.31, 6.62, and 8.62 times as high as those of corresponding elements in the surface soil in the same period, which went beyond the soil background values by more than 300% . The contribution of human activities to dustfall trace heavy metals content in Beijing city was larger than that in the surrounding region. Then sources analysis of dustfall and its 20 main trace elements (Cd, Mo, Nb, Ga, Co, Y, Nd, Li, La, Ni, Rb, V, Ce, Pb, Zr, Cr, Cu, Zn, Sr, Ba) was conducted through a multi-method analysis, including Pearson correlation analysis, Kendall correlation coefficient analysis and principal component analysis. Research results indicated that sources of winter dustfall in Beijing city were mainly composed of the earth's crust sources (including road dust, construction dust and remote transmission of dust) and the burning of fossil fuels (vehicle emissions, coal combustion, biomass combustion and industrial processes).

Resolving Molecular Clouds in the Nearby Galaxy NGC 300

NASA Astrophysics Data System (ADS)

Faesi, Christopher; Lada, Charles J.; Forbrich, Jan

2015-01-01

We present results from our ongoing Submillimeter Array (SMA) survey in which we resolve Giant Molecular Clouds (GMCs) for the first time in the nearby (D = 1.9 Mpc) spiral galaxy NGC 300. We have conducted CO(2-1) and 1.3 mm dust continuum observations of several massive star-forming regions in NGC 300, following up on the Atacama Pathfinder Experiment (APEX) survey of Faesi et al. (2014). We find that the unresolved CO sources detected with APEX at ~250 pc resolution typically resolve into one dominant GMC in our SMA observations, which have a resolution of ~3.5' (30 pc). The majority of sources are significantly detected in CO, but only one exhibits dust continuum emission. Comparing with archival H-alpha, GALEX far-ultraviolet, and Spitzer 24 micron images, we note physical offsets between the young star clusters, warm dust, and ionized and molecular gas components in these regions. We recover a widely varying fraction -- between 30% and almost 100% -- of the full APEX single dish flux with our interferometric observations. This implies that the fraction of CO-emitting molecular gas that is in a diffuse state (i.e. with characteristic spatial scales > 100 pc) differs greatly amongst star forming regions in NGC 300. We investigate potential trends in the implied diffuse molecular gas fraction with GMC properties and star formation activity. We compute virial masses and analyze the velocity structure of these resolved extragalactic GMCs and compare to results from surveys of the Milky Way and other nearby galaxies.

Dust-associated microbiomes from dryland wheat fields differ with tillage practice and biosolids application

NASA Astrophysics Data System (ADS)

Schlatter, Daniel C.; Schillinger, William F.; Bary, Andy I.; Sharratt, Brenton; Paulitz, Timothy C.

2018-07-01

Wind erosion is a significant threat to the productivity and sustainability of agricultural soils. In the dryland winter wheat (Triticum aestivum L.)-fallow region of Inland Pacific Northwest of the USA (PNW), farmers increasingly use conservation tillage practices to control wind erosion. In addition, some farmers in this dry region apply municipal biosolids to soils as fertilizer and a source of stable organic matter. The impacts of soil management practices on emissions of dust microbiota to the atmosphere are understudied. We used high-throughput DNA sequencing to examine the impacts of conservation tillage and biosolids amendments on the transport of dust-associated fungal and bacterial communities during simulated high-wind events over two years at Lind, WA. The fungal and bacterial communities contained in windblown dust differed significantly with tillage (conservation vs. conventional) and fertilizer (synthetic vs. biosolids) treatments. However, the richness and diversity of fungal and bacterial communities of dust did not vary significantly with tillage or fertilizer treatments. Taxa enriched in dust from fields under conservation tillage represented many plant-associated taxa that likely grow on residue left on the soil surface, whereas taxa that were more abundant with conventional tillage were those that likely grow on buried plant residue. Dust from biosolids-amended fields harbored greater abundances of taxa that likely feed on introduced carbon. Most human-associated taxa that may pose a health risk were not present in dust after biosolids amendment, although members of Clostridiaceae were enriched with this treatment. Results show that tillage and fertilizer management practices impact the composition of bioaerosols emitted during high-wind events and have potential implications for plant and human health.